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Sample records for dynamical spin shielding

  1. Dynamic rotating-shield brachytherapy

    SciTech Connect

    Liu, Yunlong; Flynn, Ryan T.; Kim, Yusung; Yang, Wenjun; Wu, Xiaodong

    2013-12-15

    Purpose: To present dynamic rotating shield brachytherapy (D-RSBT), a novel form of high-dose-rate brachytherapy (HDR-BT) with electronic brachytherapy source, where the radiation shield is capable of changing emission angles during the radiation delivery process.Methods: A D-RSBT system uses two layers of independently rotating tungsten alloy shields, each with a 180° azimuthal emission angle. The D-RSBT planning is separated into two stages: anchor plan optimization and optimal sequencing. In the anchor plan optimization, anchor plans are generated by maximizing the D{sub 90} for the high-risk clinical-tumor-volume (HR-CTV) assuming a fixed azimuthal emission angle of 11.25°. In the optimal sequencing, treatment plans that most closely approximate the anchor plans under the delivery-time constraint will be efficiently computed. Treatment plans for five cervical cancer patients were generated for D-RSBT, single-shield RSBT (S-RSBT), and {sup 192}Ir-based intracavitary brachytherapy with supplementary interstitial brachytherapy (IS + ICBT) assuming five treatment fractions. External beam radiotherapy doses of 45 Gy in 25 fractions of 1.8 Gy each were accounted for. The high-risk clinical target volume (HR-CTV) doses were escalated such that the D{sub 2cc} of the rectum, sigmoid colon, or bladder reached its tolerance equivalent dose in 2 Gy fractions (EQD2 with α/β= 3 Gy) of 75 Gy, 75 Gy, or 90 Gy, respectively.Results: For the patients considered, IS + ICBT had an average total dwell time of 5.7 minutes/fraction (min/fx) assuming a 10 Ci{sup 192}Ir source, and the average HR-CTV D{sub 90} was 78.9 Gy. In order to match the HR-CTV D{sub 90} of IS + ICBT, D-RSBT required an average of 10.1 min/fx more delivery time, and S-RSBT required 6.7 min/fx more. If an additional 20 min/fx of delivery time is allowed beyond that of the IS + ICBT case, D-RSBT and S-RSBT increased the HR-CTV D{sub 90} above IS + ICBT by an average of 16.3 Gy and 9.1 Gy, respectively

  2. Spin-rotation and NMR shielding constants in HCl

    SciTech Connect

    Jaszuński, Michał; Repisky, Michal; Demissie, Taye B.; Komorovsky, Stanislav; Malkin, Elena; Ruud, Kenneth; Garbacz, Piotr; Jackowski, Karol; Makulski, Włodzimierz

    2013-12-21

    The spin-rotation and nuclear magnetic shielding constants are analysed for both nuclei in the HCl molecule. Nonrelativistic ab initio calculations at the CCSD(T) level of approximation show that it is essential to include relativistic effects to obtain spin-rotation constants consistent with accurate experimental data. Our best estimates for the spin-rotation constants of {sup 1}H{sup 35}Cl are C{sub Cl}  = −53.914 kHz and C{sub H}  = 42.672 kHz (for the lowest rovibrational level). For the chlorine shielding constant, the ab initio value computed including the relativistic corrections, σ(Cl) = 976.202 ppm, provides a new absolute shielding scale; for hydrogen we find σ(H) = 31.403 ppm (both at 300 K). Combining the theoretical results with our new gas-phase NMR experimental data allows us to improve the accuracy of the magnetic dipole moments of both chlorine isotopes. For the hydrogen shielding constant, including relativistic effects yields better agreement between experimental and computed values.

  3. Dynamical Analysis of the SHIELD Galaxies

    NASA Astrophysics Data System (ADS)

    McNichols, Andrew Thomas; Teich, Yaron G.; Cannon, John M.

    2015-08-01

    We present a dynamical analysis of the 12 extremely low-mass dwarf galaxies that comprise SHIELD, a product of the Arecibo Legacy Fast ALFA survey (ALFALFA). We use multi-configuration, high spatial (˜ 150 - 350 pc) and spectral (0.82 - 2.46 km s-1 ch-1) resolution data obtained from 21 cm observations conducted with the Karl G. Jansky Very Large Array. For each source, we attempt to derive an inclination-corrected rotation curve, to calculate the maximum rotation velocity (≤ 30 km s-1 for the survey population), and to further constrain the H I mass. For sources from which a sufficiently precise rotation curve can be derived, we use spatially resolved Spitzer Space Telescope 3.6 and 4.5 μm images to determine the stellar mass as a function of radius. The gaseous and stellar mass estimates are then used to decompose the total dynamical mass values and to obtain neutral gas fractions and relative baryonic content. Characterizing the kinematics of the SHIELD galaxies allows us to draw more general conclusions about the structure and dynamical evolution of low mass dwarf galaxies in the local universe.This work is a result of collaboration with the SHIELD Team and is supported by NSF grant 1211683.

  4. SHIELD: Neutral Gas Kinematics and Dynamics

    NASA Astrophysics Data System (ADS)

    McNichols, Andrew; Teich, Yaron; Cannon, John M.; SHIELD Team

    2016-01-01

    The "Survey of HI in Extremely Low-mass Dwarfs" (SHIELD) is a multiwavelength, legacy-class observational study of 12 low-mass dwarf galaxies discovered in Arecibo Legacy Fast ALFA (ALFALFA) survey data products. Here we present new results of detailed kinematic analyses of these systems using multi-configuration, high spatial (˜300 pc) and spectral (0.82 - 2.46 km s-1 ch-1) resolution HI observations from the Karl G. Jansky Very Large Array. For each source, we produce velocity fields and dispersion maps using different spatial and spectral resolution representations of the data in order to attempt derivation of an inclination-corrected rotation curve. While both two- and three-dimensional fitting techniques are employed, the comparable magnitudes of velocity dispersion and projected rotation result in degeneracies that prohibit unambiguous circular velocity solutions. We thus make multiple position-velocity cuts across each galaxy to determine the maximum circular rotation velocity (≤ 30 km-1 for the survey population). Baryonic masses are calculated using single-dish H I fluxes from Arecibo and stellar masses derived from HST and Spitzer imaging. Comparison is made with total dynamical masses estimated from the position-velocity analysis. The SHIELD galaxies are contextualized on the baryonic Tully-Fisher relation.Support for this work was provided by NSF grant AST-1211683 to JMC at Macalester College.

  5. Spin-current emission governed by nonlinear spin dynamics

    PubMed Central

    Tashiro, Takaharu; Matsuura, Saki; Nomura, Akiyo; Watanabe, Shun; Kang, Keehoon; Sirringhaus, Henning; Ando, Kazuya

    2015-01-01

    Coupling between conduction electrons and localized magnetization is responsible for a variety of phenomena in spintronic devices. This coupling enables to generate spin currents from dynamical magnetization. Due to the nonlinearity of magnetization dynamics, the spin-current emission through the dynamical spin-exchange coupling offers a route for nonlinear generation of spin currents. Here, we demonstrate spin-current emission governed by nonlinear magnetization dynamics in a metal/magnetic insulator bilayer. The spin-current emission from the magnetic insulator is probed by the inverse spin Hall effect, which demonstrates nontrivial temperature and excitation power dependences of the voltage generation. The experimental results reveal that nonlinear magnetization dynamics and enhanced spin-current emission due to magnon scatterings are triggered by decreasing temperature. This result illustrates the crucial role of the nonlinear magnon interactions in the spin-current emission driven by dynamical magnetization, or nonequilibrium magnons, from magnetic insulators. PMID:26472712

  6. Measurements of nuclear spin dynamics by spin-noise spectroscopy

    SciTech Connect

    Ryzhov, I. I.; Poltavtsev, S. V.; Kozlov, G. G.; Zapasskii, V. S.; Kavokin, K. V.; Glazov, M. M.; Vladimirova, M.; Scalbert, D.; Cronenberger, S.; Lemaître, A.; Bloch, J.

    2015-06-15

    We exploit the potential of the spin noise spectroscopy (SNS) for studies of nuclear spin dynamics in n-GaAs. The SNS experiments were performed on bulk n-type GaAs layers embedded into a high-finesse microcavity at negative detuning. In our experiments, nuclear spin polarisation initially prepared by optical pumping is monitored in real time via a shift of the peak position in the electron spin noise spectrum. We demonstrate that this shift is a direct measure of the Overhauser field acting on the electron spin. The dynamics of nuclear spin is shown to be strongly dependent on the electron concentration.

  7. Microscopic studies of nonlocal spin dynamics and spin transport (invited)

    SciTech Connect

    Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris

    2015-05-07

    Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.

  8. Spin dynamics simulations at AGS

    SciTech Connect

    Huang, H.; MacKay, W.W.; Meot, F.; Roser, T.

    2010-05-23

    To preserve proton polarization through acceleration, it is important to have a correct model of the process. It has been known that with the insertion of the two helical partial Siberian snakes in the Alternating Gradient Synchrotron (AGS), the MAD model of AGS can not deal with a field map with offset orbit. The stepwise ray-tracing code Zgoubi provides a tool to represent the real electromagnetic fields in the modeling of the optics and spin dynamics for the AGS. Numerical experiments of resonance crossing, including spin dynamics in presence of the snakes and Q-jump, have been performed in AGS lattice models, using Zgoubi. This contribution reports on various results so obtained.

  9. GIAO-DFT isotropic magnetic shielding constants and spin-spin coupling of tartaric acid in water solution

    NASA Astrophysics Data System (ADS)

    Fideles, Bruna; Oliveira, Leonardo B. A.; Colherinhas, Guilherme

    2016-01-01

    We investigate the nuclear isotropic shielding constants and spin-spin coupling for oxygen and carbons atoms of isomers of tartaric acid in gas phase and in water solutions by Monte Carlo simulation and quantum mechanics calculations using the GIAO-B3LYP approach. Solute polarization effects are included iteratively and play an important role in the quantitative determination of shielding constants. Our MP2/aug-cc-pVTZ results show substantial increases of the dipole moment in solution as compared with the gas phase results (61-221%). The solvent effects on the σ(13O) values are in general small. More appreciable solvent effects can be seen on the σ(17O) and J(Csbnd O).

  10. Polarized hyperons probe dynamics of quark spin

    SciTech Connect

    Daniel S. Carman; T. S. Harry Lee; Mac Mestayer; Reinhard Schumacher

    2007-08-01

    Researchers at Jefferson Laboratory demonstrate how two analyses of the same data provide two plausible models of spin transfer in exclusive hyperon production, yielding quite different pictures of quark spin dynamics and challenging existing theories.

  11. Spinning compact binary : Independent variables and dynamically preserved spin configurations

    SciTech Connect

    Gergely, Laszlo Arpad

    2010-04-15

    We establish the set of independent variables suitable to monitor the complicated evolution of the spinning compact binary during the inspiral. Our approach is valid up to the second post-Newtonian order, including leading order spin-orbit, spin-spin and mass quadrupole-mass monopole effects, for generic (noncircular, nonspherical) orbits. Then, we analyze the conservative spin dynamics in terms of these variables. We prove that the only binary black hole configuration allowing for spin precessions with equal angular velocities about a common instantaneous axis roughly aligned to the normal of the osculating orbit, is the equal mass and parallel (aligned or antialigned) spin configuration. This analytic result puts limitations on what particular configurations can be selected in numerical investigations of compact binary evolutions, even in those including only the last orbits of the inspiral.

  12. Coherent spin mixing dynamics in a spin-1 atomic condensate

    SciTech Connect

    Zhang Wenxian; Chang, M.-S.; Chapman, M.S.; Zhou, D.L.; You, L.

    2005-07-15

    We study the coherent off-equilibrium spin mixing inside an atomic condensate. Using mean-field theory and adopting the single-spatial-mode approximation, the condensate spin dynamics is found to be well described by that of a nonrigid pendulum and displays a variety of periodic oscillations in an external magnetic field. Our results illuminate several recent experimental observations and provide critical insights into the observation of coherent interaction-driven oscillations in a spin-1 condensate.

  13. Spin dynamics in driven composite multiferroics

    NASA Astrophysics Data System (ADS)

    Wang, Zidong; Grimson, Malcolm J.

    2015-09-01

    A spin dynamics approach has been used to study the behavior of the magnetic spins and the electric pseudo-spins in a 1-D composite multiferroic chain with a linear magneto-electric coupling at the interface. The response is investigated with either external magnetic or electric fields driving the system. The spin dynamics is based on the Landau-Lifshitz-Gilbert equation. A Gaussian white noise is later added into the dynamic process to include the thermal effects. The interface requires a closer inspection of the magneto-electric effects. Thus, we construct a 2-D ladder model to describe the behavior of the magnetic spins and the electric pseudo-spins with different magneto-electric couplings.

  14. Spin dynamics in driven composite multiferroics

    SciTech Connect

    Wang, Zidong Grimson, Malcolm J.

    2015-09-28

    A spin dynamics approach has been used to study the behavior of the magnetic spins and the electric pseudo-spins in a 1-D composite multiferroic chain with a linear magneto-electric coupling at the interface. The response is investigated with either external magnetic or electric fields driving the system. The spin dynamics is based on the Landau-Lifshitz-Gilbert equation. A Gaussian white noise is later added into the dynamic process to include the thermal effects. The interface requires a closer inspection of the magneto-electric effects. Thus, we construct a 2-D ladder model to describe the behavior of the magnetic spins and the electric pseudo-spins with different magneto-electric couplings.

  15. Dynamic-angle spinning without sidebands

    NASA Astrophysics Data System (ADS)

    Gann, S. L.; Baltisberger, J. H.; Pines, A.

    1993-07-01

    By means of rotor-synchronized π-pulses, it is possible to eliminate the spinning sidebands (while retaining their full intensity in the isotropic centerband) that usually arise in dynamic-angle spinning (DAS) NMR. The theory of this approach, dynamic-angle hopping (DAH-180), is described and illustrated with experimental results on quadrupolar nuclei. A magic-angle hopping (MAH-180) version of magic-angle spinning is also possible and can be used in a two-dimensional NMR experiment to produce sideband-free isotropic—anisotropic correlation spectra for spin- 1/2 nuclei.

  16. Toward an absolute NMR shielding scale using the spin-rotation tensor within a relativistic framework.

    PubMed

    Aucar, I Agustín; Gomez, Sergio S; Giribet, Claudia G; Aucar, Gustavo A

    2016-08-24

    One of the most influential articles showing the best way to get the absolute values of NMR magnetic shieldings, σ (non-measurables) from both accurate measurements and theoretical calculations, was published a long time ago by Flygare. His model was shown to break down when heavy atoms are involved. This fact motivated the development of new theories of nuclear spin-rotation (SR) tensors, which consider electronic relativistic effects. One was published recently by some of us. In this article we take another step further and propose three different models that generalize Flygare's model. All of them are written using four-component relativistic expressions, though the two-component relativistic SO-S term also appears in one. The first clues for these developments were built from the relationship among σ and the SR tensors within the two-component relativistic LRESC model. Besides, we had to introduce a few other well defined assumptions: (i) relativistic corrections must be included in a way to best reproduce the relationship among the (e-e) term (called "paramagnetic" within the non-relativistic domain) of σ and its equivalent part of the SR tensor, (ii) as happens in Flygare's rule, the shielding of free atoms shall be included to improve accuracy. In the highest accurate model, a new term known as Spin-orbit due to spin, SO-S (in this mechanism the spin-Zeeman Hamiltonian replaces the orbital-Zeeman Hamiltonian), is included. We show the results of the application of those models to halogen containing linear molecules. PMID:27506822

  17. Toward an absolute NMR shielding scale using the spin-rotation tensor within a relativistic framework.

    PubMed

    Aucar, I Agustín; Gomez, Sergio S; Giribet, Claudia G; Aucar, Gustavo A

    2016-08-24

    One of the most influential articles showing the best way to get the absolute values of NMR magnetic shieldings, σ (non-measurables) from both accurate measurements and theoretical calculations, was published a long time ago by Flygare. His model was shown to break down when heavy atoms are involved. This fact motivated the development of new theories of nuclear spin-rotation (SR) tensors, which consider electronic relativistic effects. One was published recently by some of us. In this article we take another step further and propose three different models that generalize Flygare's model. All of them are written using four-component relativistic expressions, though the two-component relativistic SO-S term also appears in one. The first clues for these developments were built from the relationship among σ and the SR tensors within the two-component relativistic LRESC model. Besides, we had to introduce a few other well defined assumptions: (i) relativistic corrections must be included in a way to best reproduce the relationship among the (e-e) term (called "paramagnetic" within the non-relativistic domain) of σ and its equivalent part of the SR tensor, (ii) as happens in Flygare's rule, the shielding of free atoms shall be included to improve accuracy. In the highest accurate model, a new term known as Spin-orbit due to spin, SO-S (in this mechanism the spin-Zeeman Hamiltonian replaces the orbital-Zeeman Hamiltonian), is included. We show the results of the application of those models to halogen containing linear molecules.

  18. Exciton spin dynamics in GaSe

    SciTech Connect

    Tang, Yanhao; Xie, Wei; McGuire, John A. Lai, Chih Wei; Mandal, Krishna C.

    2015-09-21

    We analyze exciton spin dynamics in GaSe under nonresonant circularly polarized optical pumping with an exciton spin-flip rate-equation model. The model reproduces polarized time-dependent photoluminescence measurements in which the initial circular polarization approaches unity even when pumping with 0.15 eV excess energy. At T = 10 K, the exciton spin relaxation exhibits a biexponential decay with sub-20 ps and >500 ps time constants, which are also reproduced by the rate-equation model assuming distinct spin-relaxation rates for hot (nonequilibrium) and cold band-edge excitons.

  19. Unusual spin dynamics in topological insulators.

    PubMed

    Dóra, Balázs; Simon, Ferenc

    2015-10-06

    The dynamic spin susceptibility (DSS) has a ubiquitous Lorentzian form around the Zeeman energy in conventional materials with weak spin orbit coupling, whose spectral width characterizes the spin relaxation rate. We show that DSS has an unusual non-Lorentzian form in topological insulators, which are characterized by strong SOC, and the anisotropy of the DSS reveals the orientation of the underlying spin texture of topological states. At zero temperature, the high frequency part of DSS is universal and increases in certain directions as ω(d-1) with d = 2 and 3 for surface states and Weyl semimetals, respectively, while for helical edge states, the interactions renormalize the exponent as d = 2K - 1 with K the Luttinger-liquid parameter. As a result, spin relaxation rate cannot be deduced from the DSS in contrast to the case of usual metals, which follows from the strongly entangled spin and charge degrees of freedom in these systems.

  20. Unusual spin dynamics in topological insulators

    NASA Astrophysics Data System (ADS)

    Dóra, Balázs; Simon, Ferenc

    2015-10-01

    The dynamic spin susceptibility (DSS) has a ubiquitous Lorentzian form around the Zeeman energy in conventional materials with weak spin orbit coupling, whose spectral width characterizes the spin relaxation rate. We show that DSS has an unusual non-Lorentzian form in topological insulators, which are characterized by strong SOC, and the anisotropy of the DSS reveals the orientation of the underlying spin texture of topological states. At zero temperature, the high frequency part of DSS is universal and increases in certain directions as ωd-1 with d = 2 and 3 for surface states and Weyl semimetals, respectively, while for helical edge states, the interactions renormalize the exponent as d = 2K - 1 with K the Luttinger-liquid parameter. As a result, spin relaxation rate cannot be deduced from the DSS in contrast to the case of usual metals, which follows from the strongly entangled spin and charge degrees of freedom in these systems.

  1. Ab initio non-relativistic spin dynamics

    SciTech Connect

    Ding, Feizhi; Goings, Joshua J.; Li, Xiaosong; Frisch, Michael J.

    2014-12-07

    Many magnetic materials do not conform to the (anti-)ferromagnetic paradigm where all electronic spins are aligned to a global magnetization axis. Unfortunately, most electronic structure methods cannot describe such materials with noncollinear electron spin on account of formally requiring spin alignment. To overcome this limitation, it is necessary to generalize electronic structure methods and allow each electron spin to rotate freely. Here, we report the development of an ab initio time-dependent non-relativistic two-component spinor (TDN2C), which is a generalization of the time-dependent Hartree-Fock equations. Propagating the TDN2C equations in the time domain allows for the first-principles description of spin dynamics. A numerical tool based on the Hirshfeld partitioning scheme is developed to analyze the time-dependent spin magnetization. In this work, we also introduce the coupling between electron spin and a homogenous magnetic field into the TDN2C framework to simulate the response of the electronic spin degrees of freedom to an external magnetic field. This is illustrated for several model systems, including the spin-frustrated Li{sub 3} molecule. Exact agreement is found between numerical and analytic results for Larmor precession of hydrogen and lithium atoms. The TDN2C method paves the way for the ab initio description of molecular spin transport and spintronics in the time domain.

  2. Ab initio non-relativistic spin dynamics

    NASA Astrophysics Data System (ADS)

    Ding, Feizhi; Goings, Joshua J.; Frisch, Michael J.; Li, Xiaosong

    2014-12-01

    Many magnetic materials do not conform to the (anti-)ferromagnetic paradigm where all electronic spins are aligned to a global magnetization axis. Unfortunately, most electronic structure methods cannot describe such materials with noncollinear electron spin on account of formally requiring spin alignment. To overcome this limitation, it is necessary to generalize electronic structure methods and allow each electron spin to rotate freely. Here, we report the development of an ab initio time-dependent non-relativistic two-component spinor (TDN2C), which is a generalization of the time-dependent Hartree-Fock equations. Propagating the TDN2C equations in the time domain allows for the first-principles description of spin dynamics. A numerical tool based on the Hirshfeld partitioning scheme is developed to analyze the time-dependent spin magnetization. In this work, we also introduce the coupling between electron spin and a homogenous magnetic field into the TDN2C framework to simulate the response of the electronic spin degrees of freedom to an external magnetic field. This is illustrated for several model systems, including the spin-frustrated Li3 molecule. Exact agreement is found between numerical and analytic results for Larmor precession of hydrogen and lithium atoms. The TDN2C method paves the way for the ab initio description of molecular spin transport and spintronics in the time domain.

  3. Density-Functional and Coupled-Cluster Singles-and-Doubles Calculations of the Nuclear Shielding and Indirect Nuclear Spin-Spin Coupling Constants of o-Benzyne.

    PubMed

    Helgaker, Trygve; Jaszuński, Michał

    2007-01-01

    Density-functional theory (DFT) and coupled-cluster singles-and-doubles (CCSD) theory are applied to compute the nuclear magnetic resonance (NMR) shielding and indirect nuclear spin-spin coupling constants of o-benzyne, whose biradical nature makes it difficult to study both experimentally and theoretically. Because of near-equilibrium triplet instabilities that follow from its biradical character, the calculated DFT NMR properties of o-benzyne are unusually sensitive to details of the exchange-correlation functional. However, this sensitivity is greatly reduced if these properties are calculated at the equilibrium of the chosen functional. A strong correlation is demonstrated between the quality of the calculated indirect spin-spin coupling constants and the quality of the calculated lowest triplet excitation energy in o-benzyne. Orbital-unrelaxed coupled-cluster theory should be less affected by such instabilities, and the CCSD NMR properties were only calculated at the experimental equilibrium geometry. For the shielding constants, the results in best agreement with experimental results are obtained with CCSD theory and with the Keal-Tozer KT1 and KT2 functionals. For the triply bonded carbon atoms, these models yield an isotropic shielding of 1.3, -3.3, and -1.2 ppm, respectively, compared with the experimentally observed shielding of 3.7 ppm for incarcerated o-benzyne. For the indirect spin-spin coupling constants, the CCSD model and the Perdew-Burke-Ernzerhof functional both yield reliable results; for the most interesting spin-spin coupling constant, (1)J (C⋮C), we obtain 210 and 209 Hz with these two models, respectively, somewhat above the recently reported experimental value of 177.9 ± 0.7 Hz for o-benzyne inside a molecular container, suggesting large incarceration effects.

  4. Dynamic spin susceptibility of interacting electron systems

    NASA Astrophysics Data System (ADS)

    Zyuzin, Vladimir; Maslov, Dmitrii

    2015-03-01

    We study the dynamic spin susceptibility of interacting electrons in spatial dimensions from one to three. In all cases, backscattering processes result in non-zero imaginary part of the spin susceptibility above the particle-hole continuum of non-interacting electrons. In one dimension, we employ the renormalization group to go beyond the second order and obtain a general expression for the spin susceptibility. In higher dimensions, we show that the imaginary part of the spin susceptibility arises from the same mechanism as non-analytic corrections to the Fermi-liquid theory. We relate the obtained results to the lifetime of collective spin modes. This work was supported by the National Science Foundation via Grant NSF DMR-1308972.

  5. Spinning compact binary dynamics and chameleon orbits

    NASA Astrophysics Data System (ADS)

    Gergely, László Árpád; Keresztes, Zoltán

    2015-01-01

    We analyze the conservative evolution of spinning compact binaries to second post-Newtonian (2PN) order accuracy, with leading-order spin-orbit, spin-spin and mass quadrupole-monopole contributions included. As a main result we derive a closed system of first-order differential equations in a compact form, for a set of dimensionless variables encompassing both orbital elements and spin angles. These evolutions are constrained by conservation laws holding at 2PN order. As required by the generic theory of constrained dynamical systems we perform a consistency check and prove that the constraints are preserved by the evolution. We apply the formalism to show the existence of chameleon orbits, whose local, orbital parameters evolve from elliptic (in the Newtonian sense) near pericenter, towards hyperbolic at large distances. This behavior is consistent with the picture that general relativity predicts stronger gravity at short distances than Newtonian theory does.

  6. Magnetic Suspension for Dynamic Spin Rig

    NASA Technical Reports Server (NTRS)

    Johnson, Dexter

    1998-01-01

    NASA Lewis Research Center's Dynamic Spin Rig, located in Building 5, Test Cell CW-18, is used to test turbomachinery blades and components by rotating them in a vacuum chamber. A team from Lewis' Machine Dynamics Branch successfully integrated a magnetic bearing and control system into the Dynamic Spin Rig. The magnetic bearing worked very well both to support and shake the shaft. It was demonstrated that the magnetic bearing can transmit more vibrational energy into the shaft and excite some blade modes to larger amplitudes than the existing electromagnetic shakers can.

  7. Atomistic spin dynamics and surface magnons.

    PubMed

    Etz, Corina; Bergqvist, Lars; Bergman, Anders; Taroni, Andrea; Eriksson, Olle

    2015-06-24

    Atomistic spin dynamics simulations have evolved to become a powerful and versatile tool for simulating dynamic properties of magnetic materials. It has a wide range of applications, for instance switching of magnetic states in bulk and nano-magnets, dynamics of topological magnets, such as skyrmions and vortices and domain wall motion. In this review, after a brief summary of the existing investigation tools for the study of magnons, we focus on calculations of spin-wave excitations in low-dimensional magnets and the effect of relativistic and temperature effects in such structures. In general, we find a good agreement between our results and the experimental values. For material specific studies, the atomistic spin dynamics is combined with electronic structure calculations within the density functional theory from which the required parameters are calculated, such as magnetic exchange interactions, magnetocrystalline anisotropy, and Dzyaloshinskii-Moriya vectors. PMID:26030259

  8. Fine-tuning the etch depth profile via dynamic shielding of ion beam

    NASA Astrophysics Data System (ADS)

    Wu, Lixiang; Qiu, Keqiang; Fu, Shaojun

    2016-08-01

    We introduce a method for finely adjusting the etch depth profile by dynamic shielding in the course of ion beam etching (IBE), which is crucial for the ultra-precision fabrication of large optics. We study the physical process of dynamic shielding and propose a parametric modeling method to quantitatively analyze the shielding effect on etch depths, or rather the shielding rate, where a piecewise Gaussian model is adopted to fit the shielding rate profile. Two experiments were conducted. The experimental result of parametric modeling of shielding rate profiles shows that the shielding rate profile is significantly influenced by the rotary angle of the leaf. The result of the experiment on fine-tuning the etch depth profile shows good agreement with the simulated result, which preliminarily verifies the feasibility of our method.

  9. Spin Hall phenomenology of magnetic dynamics

    NASA Astrophysics Data System (ADS)

    Tserkovnyak, Yaroslav; Bender, Scott A.

    2014-07-01

    We study the role of spin-orbit interactions in the coupled magnetoelectric dynamics of a ferromagnetic film coated with an electrical conductor. While the main thrust of this work is phenomenological, several popular simple models are considered microscopically in some detail, including Rashba and Dirac two-dimensional electron gases coupled to a magnetic insulator, as well as a diffusive spin Hall system. We focus on the long-wavelength magnetic dynamics that experiences current-induced torques and produces fictitious electromotive forces. Our phenomenology provides a suitable framework for analyzing experiments on current-induced magnetic dynamics and reciprocal charge pumping, including the effects of magnetoresistance and Gilbert-damping anisotropies, without a need to resort to any microscopic considerations or modeling. Finally, some remarks are made regarding the interplay of spin-orbit interactions and magnetic textures.

  10. Spin dynamics in geometrically frustrated antiferromagnetic pyrochlores

    NASA Astrophysics Data System (ADS)

    Gardner, J. S.; Ehlers, G.; Bramwell, S. T.; Gaulin, B. D.

    2004-03-01

    We have studied the spin dynamics of several antiferromagnetic pyrochlore oxides. These magnets are geometrically frustrated and only reach their ground states at temperatures much lower than that expected from mean field theory. Here we present data on the magnetic nature, especially the spin dynamics of Tb2Ti2O7, Gd2Ti2O7 and Y2Mo2O7. In these systems the ground states are found to be very different. Y2Mo2O7 freezes completely into a spin glass-like state, Tb2Ti2O7 is a cooperative paramagnetic and remains dynamic down to 15 mK and Gd2Ti2O7 enters a unique partially ordered state at {\\sim }1 K.

  11. Investigation of triple spin correlations and spin dynamics in ferromagnets

    SciTech Connect

    Okorokov, A. I.

    2011-12-15

    Data on the experimental detection and use of three-particle (chiral) spin dynamic correlations in ferromagnets are presented. The oblique-geometry method for investigating polarized neutron small-angle scattering is described, which gives the dependence that the scattering asymmetry has on the polarization P signs and the scattering angle {theta}. The following results of the dynamics investigation in the critical and ferromagnetic phases in the magnetic field are presented: the temperature dependence of the critical field H{sub c}, the factorization of the momentum transfer dependence of three-particle vertices, the corroboration of the 'hard' version of the dipole critical dynamics, and the dynamics of amorphous magnets and invars.

  12. Spin dynamics on percolating networks

    SciTech Connect

    Aeppli, G.; Guggenheim, H.; Uemura, Y.J.

    1985-01-01

    We have used inelastic neutron scattering to measure the order parameter relaxation rate GAMMA in the dilute, two-dimensional Ising antiferromagnet Rb/sub 2/CoMg/sub 1-c/F/sub 4/ with c very close to the magnetic percolation threshold. Where kappa is the inverse magnetic correlation length, GAMMA approx. kappa/sup z/ with z = 2.4/sub -0.1//sup +0.2/. Our results are discussed in terms of current ideas about spin relaxation on fractals. 13 refs., 1 fig.

  13. The classical and quantum dynamics of molecular spins on graphene.

    PubMed

    Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo

    2016-02-01

    Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic and quantum computing devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics and electrical spin manipulation. However, the influence of the graphene environment on the spin systems has yet to be unravelled. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets on graphene. Whereas the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly developed model. Coupling to Dirac electrons introduces a dominant quantum relaxation channel that, by driving the spins over Villain's threshold, gives rise to fully coherent, resonant spin tunnelling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin manipulation in graphene nanodevices. PMID:26641019

  14. RNA Dynamics: Perspectives from Spin Labels

    PubMed Central

    Nguyen, Phuong

    2011-01-01

    Dynamics are an important and indispensible physical attribute that plays essential roles in RNA function. RNA dynamics are complex, spanning vast timescales and encompassing large number of physical modes. The technique of site-directed spin labeling (SDSL), which derives information on local structural and dynamic features of a macromolecule by monitoring a chemically stable nitroxide radical using electron paramagnetic resonance (EPR) spectroscopy, has been applied to monitor intrinsic dynamics at defined structural states as well as to probe conformational transition dynamics of RNAs. Current state of SDSL studies of RNA dynamics is summarized here. Further SDSL developments promise to open up many more opportunities for probing RNA dynamics and connecting dynamics to structure and function. PMID:21882345

  15. Unusual spin dynamics in topological insulators

    PubMed Central

    Dóra, Balázs; Simon, Ferenc

    2015-01-01

    The dynamic spin susceptibility (DSS) has a ubiquitous Lorentzian form around the Zeeman energy in conventional materials with weak spin orbit coupling, whose spectral width characterizes the spin relaxation rate. We show that DSS has an unusual non-Lorentzian form in topological insulators, which are characterized by strong SOC, and the anisotropy of the DSS reveals the orientation of the underlying spin texture of topological states. At zero temperature, the high frequency part of DSS is universal and increases in certain directions as ωd−1 with d = 2 and 3 for surface states and Weyl semimetals, respectively, while for helical edge states, the interactions renormalize the exponent as d = 2K − 1 with K the Luttinger-liquid parameter. As a result, spin relaxation rate cannot be deduced from the DSS in contrast to the case of usual metals, which follows from the strongly entangled spin and charge degrees of freedom in these systems. PMID:26439629

  16. Spin dynamics in the multiferroic materials (invited)

    SciTech Connect

    Ye, Feng; Fishman, Randy Scott; Haraldsen, Jason T; Lorenz, Bernd; Chu, C. W.; Kimura, K.

    2012-01-01

    We report high resolution inelastic neutron scattering measurements and spin dynamics calculations in two multiferroic materials: the geometrically frustrated triangular lattice CuFeO2 and mineral Hu bnerite MnWO4. In un-doped CuFeO2 a low-T collinear spin structure is stabilized by long range magnetic interactions. When doped with a few percent of gallium, the spin order evolves into a complex noncollinear configuration and the system becomes multiferroic. Similarly, the ground state collinear spin order in pure MnWO4 results from delicate balance between competing magnetic interactions up to 11th nearest neighbors and can be tuned by substitution of Mn ions with magnetic or nonmagnetic impurities. The comprehensive investigation of spin dynamics in both systems help to understand the fundamental physical process and the interactions leading to the close interplay of magnetism and ferroelectricity in this type of materials. VC2012 American Institute of Physics. [doi:10.1063/1.3677863

  17. Longitudinal spin dynamics in ferrimagnets: Multiple spin wave nature of longitudinal spin excitations

    NASA Astrophysics Data System (ADS)

    Krivoruchko, V. N.

    2016-08-01

    Motivated by the existing controversy about the physical mechanisms that govern longitudinal magnetization dynamics under the effect of ultrafast laser pulses, in this paper we study the microscopic model of longitudinal spin excitations in a two-sublattice ferrimagnet using the diagrammatic technique for spin operators. The diagrammatic approach provides us with an efficient procedure to derive graphical representations for perturbation expansion series for different spin Green's functions and thus to overcome limitations typical for phenomenological approaches. The infinite series involving all distinct loops built from spin wave propagators are summed up. These result in an expression for the longitudinal spin susceptibility χz z(q ,ω ) applicable in all regions of frequency ω and wave vector q space beyond the hydrodynamical and critical regimes. A strong renormalization of the longitudinal spin oscillations due to processes of virtual creation and annihilation of transverse spin waves has been found. We have shown that the spectrum of longitudinal excitations consists of a quasirelaxation mode forming a central peak in χz z(q ,ω ) and two (acoustic and exchange) precessionlike modes. As the main result, it is predicted that both acoustic and exchange longitudinal excitations are energetically above similar modes of transverse spin waves at the same temperature and wave vector. The existence of the exchange longitudinal mode at such frequencies can result in a new form of excitation behavior in ferrimagnetic system, which could be important for understanding the physics of nonequilibrium magnetic dynamics under the effect of ultrafast laser pulses in multisublattice magnetic materials.

  18. Dynamic Feedback in Ferromagnet-Spin Hall Metal Heterostructures

    NASA Astrophysics Data System (ADS)

    Cheng, Ran; Zhu, Jian-Gang; Xiao, Di

    2016-08-01

    In ferromagnet-normal-metal heterostructures, spin pumping and spin-transfer torques are two reciprocal processes that occur concomitantly. Their interplay introduces a dynamic feedback effect interconnecting energy dissipation channels of both magnetization and current. By solving the spin diffusion process in the presence of the spin Hall effect in the normal metal, we show that the dynamic feedback gives rise to (i) a nonlinear magnetic damping that is crucial to sustain uniform steady-state oscillations of a spin Hall oscillator at large angles and (ii) a frequency-dependent spin Hall magnetoimpedance that reduces to the spin Hall magnetoresistance in the dc limit.

  19. Dynamic Feedback in Ferromagnet-Spin Hall Metal Heterostructures.

    PubMed

    Cheng, Ran; Zhu, Jian-Gang; Xiao, Di

    2016-08-26

    In ferromagnet-normal-metal heterostructures, spin pumping and spin-transfer torques are two reciprocal processes that occur concomitantly. Their interplay introduces a dynamic feedback effect interconnecting energy dissipation channels of both magnetization and current. By solving the spin diffusion process in the presence of the spin Hall effect in the normal metal, we show that the dynamic feedback gives rise to (i) a nonlinear magnetic damping that is crucial to sustain uniform steady-state oscillations of a spin Hall oscillator at large angles and (ii) a frequency-dependent spin Hall magnetoimpedance that reduces to the spin Hall magnetoresistance in the dc limit. PMID:27610880

  20. Dynamics of the Lunar Spin Axis

    NASA Technical Reports Server (NTRS)

    Wisdom, Jack

    2006-01-01

    The evolution of the lunar spin axis is studied. Prior work has assumed that the inclination of the lunar orbit is constant and that the node regresses uniformly. This work takes into account the nonconstant inclination and nonuniform regression of the node as determined from averaged models of the motion of the lunar orbit. The resulting dynamics is considerably more rich, exhibiting additional resonances, period doubling and tripling, and chaos.

  1. Combined molecular dynamics-spin dynamics simulations of bcc iron

    SciTech Connect

    Perera, Meewanage Dilina N; Yin, Junqi; Landau, David P; Nicholson, Don M; Stocks, George Malcolm; Eisenbach, Markus; Brown, Greg

    2014-01-01

    Using a classical model that treats translational and spin degrees of freedom on an equal footing, we study phonon-magnon interactions in BCC iron with combined molecular and spin dynamics methods. The atomic interactions are modeled via an empirical many-body potential while spin dependent interactions are established through a Hamiltonian of the Heisenberg form with a distance dependent magnetic exchange interaction obtained from first principles electronic structure calculations. The temporal evolution of translational and spin degrees of freedom was determined by numerically solving the coupled equations of motion, using an algorithm based on the second order Suzuki-Trotter decomposition of the exponential operators. By calculating Fourier transforms of space- and time-displaced correlation functions, we demonstrate that the the presence of lattice vibrations leads to noticeable softening and damping of spin wave modes. As a result of the interplay between lattice and spin subsystems, we also observe additional longitudinal spin wave excitations, with frequencies which coincide with that of the longitudinal lattice vibrations.

  2. Theoretical prediction of nuclear magnetic shieldings and indirect spin-spin coupling constants in 1,1-, cis-, and trans-1,2-difluoroethylenes

    SciTech Connect

    Nozirov, Farhod E-mail: farhod.nozirov@gmail.com; Stachów, Michał; Kupka, Teobald E-mail: farhod.nozirov@gmail.com

    2014-04-14

    A theoretical prediction of nuclear magnetic shieldings and indirect spin-spin coupling constants in 1,1-, cis- and trans-1,2-difluoroethylenes is reported. The results obtained using density functional theory (DFT) combined with large basis sets and gauge-independent atomic orbital calculations were critically compared with experiment and conventional, higher level correlated electronic structure methods. Accurate structural, vibrational, and NMR parameters of difluoroethylenes were obtained using several density functionals combined with dedicated basis sets. B3LYP/6-311++G(3df,2pd) optimized structures of difluoroethylenes closely reproduced experimental geometries and earlier reported benchmark coupled cluster results, while BLYP/6-311++G(3df,2pd) produced accurate harmonic vibrational frequencies. The most accurate vibrations were obtained using B3LYP/6-311++G(3df,2pd) with correction for anharmonicity. Becke half and half (BHandH) density functional predicted more accurate {sup 19}F isotropic shieldings and van Voorhis and Scuseria's τ-dependent gradient-corrected correlation functional yielded better carbon shieldings than B3LYP. A surprisingly good performance of Hartree-Fock (HF) method in predicting nuclear shieldings in these molecules was observed. Inclusion of zero-point vibrational correction markedly improved agreement with experiment for nuclear shieldings calculated by HF, MP2, CCSD, and CCSD(T) methods but worsened the DFT results. The threefold improvement in accuracy when predicting {sup 2}J(FF) in 1,1-difluoroethylene for BHandH density functional compared to B3LYP was observed (the deviations from experiment were −46 vs. −115 Hz)

  3. Dynamic Open-Rotor Composite Shield Impact Test Report

    NASA Technical Reports Server (NTRS)

    Seng, Silvia; Frankenberger, Charles; Ruggeri, Charles R.; Revilock, Duane M.; Pereira, J. Michael; Carney, Kelly S.; Emmerling, William C.

    2015-01-01

    The Federal Aviation Administration (FAA) is working with the European Aviation Safety Agency to determine the certification base for proposed new engines that would not have a containment structure on large commercial aircraft. Equivalent safety to the current fleet is desired by the regulators, which means that loss of a single fan blade will not cause hazard to the aircraft. NASA Glenn and Naval Air Warfare Center (NAWC) China Lake collaborated with the FAA Aircraft Catastrophic Failure Prevention Program to design and test a shield that would protect the aircraft passengers and critical systems from a released blade that could impact the fuselage. This report documents the live-fire test from a full-scale rig at NAWC China Lake. NASA provided manpower and photogrammetry expertise to document the impact and damage to the shields. The test was successful: the blade was stopped from penetrating the shield, which validates the design analysis method and the parameters used in the analysis. Additional work is required to implement the shielding into the aircraft.

  4. Entanglement Dynamics of Two Spins in Initially Correlated Wheel-Shaped Spin Baths

    NASA Astrophysics Data System (ADS)

    Sun, Kai-Le; Chen, Jun; Wang, Fa-Qiang; Yu, Ya-Fei; Zhang, Zhi-Ming

    2016-02-01

    We study the effects of the initial correlations in environment on the entanglement dynamics of spin system. The correlated environment is novelly simulated by two correlated wheel-shaped spin baths, each consisting of an intermediate spin interacting with a spin-ring. The correlations in environment are achieved by the entanglement between two intermediate spins. The spin system includes two system-spins, and the interaction between the spin system and the environment is implemented by the coupling between the system-spin and the intermediate spin. Firstly, we analyze the influences of the initial entanglement between the two intermediate spins, the coupling parameters and the temperature of the baths on the entanglement dynamics of the two system-spins in equivalent subsystems. It is demonstrated that the initial entanglement between the baths can act as a resource for the generation and the revivals of the entanglement of the system-spins. Moreover, the amount of the generation and the revivals of the entanglement of the system-spins can be enhanced by regulating the coupling constants and the temperature of the baths. In addition, we also investigate the influences of different coupling ratios in non-equivalent subsystems, it is found that changing the coupling ratios of two subsystems has a significant effect on the generation and revivals of entanglement of system-spins.

  5. Momentum and spin in entropic quantum dynamics

    NASA Astrophysics Data System (ADS)

    Nawaz, Shahid

    We study quantum theory as an example of entropic inference. Our goal is to remove conceptual difficulties that arise in quantum mechanics. Since probability is a common feature of quantum theory and of any inference problem, we briefly introduce probability theory and the entropic methods to update probabilities when new information becomes available. Nelson's stochastic mechanics and Caticha's derivation of quantum theory are discussed in the subsequent chapters. Our first goal is to understand momentum and angular momentum within an entropic dynamics framework and to derive the corresponding uncertainty relations. In this framework momentum is an epistemic concept -- it is not an attribute of the particle but of the probability distributions. We also show that the Heisenberg's uncertainty relation is an osmotic effect. Next we explore the entropic analog of angular momentum. Just like linear momentum, angular momentum is also expressed in purely informational terms. We then extend entropic dynamics to curved spaces. An important new feature is that the displacement of a particle does not transform like a vector. It involves second order terms that account for the effects of curvature . This leads to a modified Schrodinger equation for curved spaces that also take into account the curvature effects. We also derive Schrodinger equation for a charged particle interacting with external electromagnetic field on general Riemannian manifolds. Finally we develop the entropic dynamics of a particle of spin 1/2. The particle is modeled as a rigid point rotator interacting with an external EM field. The configuration space of such a rotator is R 3 x S3 (S 3 is the 3-sphere). The model describes the regular representation of SU(2) which includes all the irreducible representations (spin 0, 1/2, 1, 3/2,...) including spin 1/2.

  6. Spinning compact binary inspiral. II. Conservative angular dynamics

    SciTech Connect

    Gergely, Laszlo Arpad

    2010-11-15

    We establish the evolution equations of the set of independent variables characterizing the 2PN rigorous conservative dynamics of a spinning compact binary, with the inclusion of the leading order spin-orbit, spin-spin, and mass quadrupole-mass monopole effects, for generic (noncircular, nonspherical) orbits. More specifically, we give a closed system of first order ordinary differential equations for the orbital elements of the osculating ellipse and for the angles characterizing the spin orientations with respect to the osculating orbit. We also prove that (i) the relative angle of the spins stays constant for equal mass black holes, irrespective of their orientation, and (ii) the special configuration of equal mass black holes with equal, but antialigned spins, both laying in the plane of motion (leading to the largest recoil found in numerical simulations) is preserved at 2PN level of accuracy, with leading order spin-orbit, spin-spin, and mass quadrupolar contributions included.

  7. Shielding and indirect spin-spin coupling tensors in the presence of a heavy atom: an experimental and theoretical study of bis(phenylethynyl)mercury.

    PubMed

    Gryff-Keller, Adam; Kraska-Dziadecka, Anna; Molchanov, Sergey; Wodyński, Artur

    2012-11-01

    Magnetic shielding and indirect spin-spin coupling phenomena are tensorial properties and both their isotropic and anisotropic parts do affect NMR spectra. The involved interaction tensors, σ and J, can nowadays be theoretically calculated, although the reliability of such methods in the case of anisotropic parameters, Δσ and ΔJ, in systems involving heavy nuclei, yet demands testing. In this communication the results of the experimental and theoretical investigations of bis(phenylethynyl)mercury (I) labeled with (13)C isotope at positions neighboring Hg are reported. The theoretical calculations of molecular geometry and values of NMR parameters for I have been performed by the ZORA/DFT method, including the relativistic scalar and spin-orbit coupling contributions, using the PBE0 functional and TZP (or jcpl) basis set. These values have been confronted with the experimentally measured ones. The isotropic parameters have been measured by the standard (13)C and (199)Hg NMR spectra. The shielding anisotropies for the atoms in the central part of molecule I have been determined in a liquid sample using magnetic relaxation measurements. The relaxation data have been interpreted within the rotational diffusion theory, assuming the symmetrical top reorientation model. The anisotropies of one-bond (13)C-(199)Hg and two-bond (13)C-Hg-(13)C spin-spin couplings have been determined exploiting the temperature-dependent (13)C NMR spectra of I in the ZLI1167 liquid-crystal phase. We have found that our theoretical calculations reproduce experimental values of both isotropic and anisotropic NMR parameters very well.

  8. Current-driven spin dynamics of artificially constructed quantum magnets.

    PubMed

    Khajetoorians, Alexander Ako; Baxevanis, Benjamin; Hübner, Christoph; Schlenk, Tobias; Krause, Stefan; Wehling, Tim Oliver; Lounis, Samir; Lichtenstein, Alexander; Pfannkuche, Daniela; Wiebe, Jens; Wiesendanger, Roland

    2013-01-01

    The future of nanoscale spin-based technologies hinges on a fundamental understanding and dynamic control of atomic-scale magnets. The role of the substrate conduction electrons on the dynamics of supported atomic magnets is still a question of interest lacking experimental insight. We characterized the temperature-dependent dynamical response of artificially constructed magnets, composed of a few exchange-coupled atomic spins adsorbed on a metallic substrate, to spin-polarized currents driven and read out by a magnetic scanning tunneling microscope tip. The dynamics, reflected by two-state spin noise, is quantified by a model that considers the interplay between quantum tunneling and sequential spin transitions driven by electron spin-flip processes and accounts for an observed spin-transfer torque effect.

  9. Simulating electron spin resonance spectra of nitroxide spin labels from molecular dynamics and stochastic trajectories

    PubMed Central

    Sezer, Deniz; Freed, Jack H.; Roux, Benoît

    2008-01-01

    Simulating electron spin resonance spectra of nitroxide spin labels from motional models is necessary for the quantitative analysis of experimental spectra. We present a framework for modeling the spin label dynamics by using trajectories such as those from molecular dynamics (MD) simulations combined with stochastic treatment of the global protein tumbling. This is achieved in the time domain after two efficient numerical integrators are developed: One for the quantal dynamics of the spins and the other for the classical rotational diffusion. For the quantal dynamics, we propagate the relevant part of the spin density matrix in Hilbert space. For the diffusional tumbling, we work with quaternions, which enables the treatment of anisotropic diffusion in a potential expanded as a sum of spherical harmonics. Time-averaging arguments are invoked to bridge the gap between the smaller time step of the MD trajectories and the larger time steps appropriate for the rotational diffusion and∕or quantal spin dynamics. PMID:18447510

  10. Nonequilibrium Spin Dynamics in a Trapped Fermi Gas with Effective Spin-Orbit Interactions

    SciTech Connect

    Stanescu, Tudor D.; Zhang Chuanwei; Galitski, Victor

    2007-09-14

    We consider a trapped atomic system in the presence of spatially varying laser fields. The laser-atom interaction generates a pseudospin degree of freedom (referred to simply as spin) and leads to an effective spin-orbit coupling for the fermions in the trap. Reflections of the fermions from the trap boundaries provide a physical mechanism for effective momentum relaxation and nontrivial spin dynamics due to the emergent spin-orbit coupling. We explicitly consider evolution of an initially spin-polarized Fermi gas in a two-dimensional harmonic trap and derive nonequilibrium behavior of the spin polarization. It shows periodic echoes with a frequency equal to the harmonic trapping frequency. Perturbations, such as an asymmetry of the trap, lead to the suppression of the spin echo amplitudes. We discuss a possible experimental setup to observe spin dynamics and provide numerical estimates of relevant parameters.

  11. Dynamic Stabilization of a Quantum Many-Body Spin System

    NASA Astrophysics Data System (ADS)

    Hoang, T. M.; Gerving, C. S.; Land, B. J.; Anquez, M.; Hamley, C. D.; Chapman, M. S.

    2013-08-01

    We demonstrate dynamic stabilization of a strongly interacting quantum spin system realized in a spin-1 atomic Bose-Einstein condensate. The spinor Bose-Einstein condensate is initialized to an unstable fixed point of the spin-nematic phase space, where subsequent free evolution gives rise to squeezing and quantum spin mixing. To stabilize the system, periodic microwave pulses are applied that rotate the spin-nematic many-body fluctuations and limit their growth. The stability diagram for the range of pulse periods and phase shifts that stabilize the dynamics is measured and compares well with a stability analysis.

  12. Dynamic stabilization of a quantum many-body spin system.

    PubMed

    Hoang, T M; Gerving, C S; Land, B J; Anquez, M; Hamley, C D; Chapman, M S

    2013-08-30

    We demonstrate dynamic stabilization of a strongly interacting quantum spin system realized in a spin-1 atomic Bose-Einstein condensate. The spinor Bose-Einstein condensate is initialized to an unstable fixed point of the spin-nematic phase space, where subsequent free evolution gives rise to squeezing and quantum spin mixing. To stabilize the system, periodic microwave pulses are applied that rotate the spin-nematic many-body fluctuations and limit their growth. The stability diagram for the range of pulse periods and phase shifts that stabilize the dynamics is measured and compares well with a stability analysis. PMID:24033006

  13. Dynamical cancellation of pulse-induced transients in a metallic shielded room for ultra-low-field magnetic resonance imaging

    NASA Astrophysics Data System (ADS)

    Zevenhoven, Koos C. J.; Dong, Hui; Ilmoniemi, Risto J.; Clarke, John

    2015-01-01

    Pulse-induced transients such as eddy currents can cause problems in measurement techniques where a signal is acquired after an applied preparatory pulse. In ultra-low-field magnetic resonance imaging, performed in magnetic fields typically of the order of 100 μT, the signal-to-noise ratio is enhanced in part by prepolarizing the proton spins with a pulse of much larger magnetic field and in part by detecting the signal with a Superconducting QUantum Interference Device (SQUID). The pulse turn-off, however, can induce large eddy currents in the shielded room, producing an inhomogeneous magnetic-field transient that both seriously distorts the spin dynamics and exceeds the range of the SQUID readout. It is essential to reduce this transient substantially before image acquisition. We introduce dynamical cancellation (DynaCan), a technique in which a precisely designed current waveform is applied to a separate coil during the later part and turn off of the polarizing pulse. This waveform, which bears no resemblance to the polarizing pulse, is designed to drive the eddy currents to zero at the precise moment that the polarizing field becomes zero. We present the theory used to optimize the waveform using a detailed computational model with corrections from measured magnetic-field transients. SQUID-based measurements with DynaCan demonstrate a cancellation of 99%. Dynamical cancellation has the great advantage that, for a given system, the cancellation accuracy can be optimized in software. This technique can be applied to both metal and high-permeability alloy shielded rooms, and even to transients other than eddy currents.

  14. Dynamical cancellation of pulse-induced transients in a metallic shielded room for ultra-low-field magnetic resonance imaging

    SciTech Connect

    Zevenhoven, Koos C. J. Ilmoniemi, Risto J.; Dong, Hui; Clarke, John

    2015-01-19

    Pulse-induced transients such as eddy currents can cause problems in measurement techniques where a signal is acquired after an applied preparatory pulse. In ultra-low-field magnetic resonance imaging, performed in magnetic fields typically of the order of 100 μT, the signal-to-noise ratio is enhanced in part by prepolarizing the proton spins with a pulse of much larger magnetic field and in part by detecting the signal with a Superconducting QUantum Interference Device (SQUID). The pulse turn-off, however, can induce large eddy currents in the shielded room, producing an inhomogeneous magnetic-field transient that both seriously distorts the spin dynamics and exceeds the range of the SQUID readout. It is essential to reduce this transient substantially before image acquisition. We introduce dynamical cancellation (DynaCan), a technique in which a precisely designed current waveform is applied to a separate coil during the later part and turn off of the polarizing pulse. This waveform, which bears no resemblance to the polarizing pulse, is designed to drive the eddy currents to zero at the precise moment that the polarizing field becomes zero. We present the theory used to optimize the waveform using a detailed computational model with corrections from measured magnetic-field transients. SQUID-based measurements with DynaCan demonstrate a cancellation of 99%. Dynamical cancellation has the great advantage that, for a given system, the cancellation accuracy can be optimized in software. This technique can be applied to both metal and high-permeability alloy shielded rooms, and even to transients other than eddy currents.

  15. SD-CAS: Spin Dynamics by Computer Algebra System.

    PubMed

    Filip, Xenia; Filip, Claudiu

    2010-11-01

    A computer algebra tool for describing the Liouville-space quantum evolution of nuclear 1/2-spins is introduced and implemented within a computational framework named Spin Dynamics by Computer Algebra System (SD-CAS). A distinctive feature compared with numerical and previous computer algebra approaches to solving spin dynamics problems results from the fact that no matrix representation for spin operators is used in SD-CAS, which determines a full symbolic character to the performed computations. Spin correlations are stored in SD-CAS as four-entry nested lists of which size increases linearly with the number of spins into the system and are easily mapped into analytical expressions in terms of spin operator products. For the so defined SD-CAS spin correlations a set of specialized functions and procedures is introduced that are essential for implementing basic spin algebra operations, such as the spin operator products, commutators, and scalar products. They provide results in an abstract algebraic form: specific procedures to quantitatively evaluate such symbolic expressions with respect to the involved spin interaction parameters and experimental conditions are also discussed. Although the main focus in the present work is on laying the foundation for spin dynamics symbolic computation in NMR based on a non-matrix formalism, practical aspects are also considered throughout the theoretical development process. In particular, specific SD-CAS routines have been implemented using the YACAS computer algebra package (http://yacas.sourceforge.net), and their functionality was demonstrated on a few illustrative examples.

  16. SD-CAS: Spin Dynamics by Computer Algebra System

    NASA Astrophysics Data System (ADS)

    Filip, Xenia; Filip, Claudiu

    2010-11-01

    A computer algebra tool for describing the Liouville-space quantum evolution of nuclear 1/2-spins is introduced and implemented within a computational framework named Spin Dynamics by Computer Algebra System (SD-CAS). A distinctive feature compared with numerical and previous computer algebra approaches to solving spin dynamics problems results from the fact that no matrix representation for spin operators is used in SD-CAS, which determines a full symbolic character to the performed computations. Spin correlations are stored in SD-CAS as four-entry nested lists of which size increases linearly with the number of spins into the system and are easily mapped into analytical expressions in terms of spin operator products. For the so defined SD-CAS spin correlations a set of specialized functions and procedures is introduced that are essential for implementing basic spin algebra operations, such as the spin operator products, commutators, and scalar products. They provide results in an abstract algebraic form: specific procedures to quantitatively evaluate such symbolic expressions with respect to the involved spin interaction parameters and experimental conditions are also discussed. Although the main focus in the present work is on laying the foundation for spin dynamics symbolic computation in NMR based on a non-matrix formalism, practical aspects are also considered throughout the theoretical development process. In particular, specific SD-CAS routines have been implemented using the YACAS computer algebra package (http://yacas.sourceforge.net), and their functionality was demonstrated on a few illustrative examples.

  17. The classical and quantum dynamics of molecular spins on graphene

    PubMed Central

    Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo

    2015-01-01

    Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic1 and quantum computing2 devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics3,4, and electrical spin-manipulation4-11. However, the influence of the graphene environment on the spin systems has yet to be unraveled12. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets13 on graphene. While the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly-developed model. Coupling to Dirac electrons introduces a dominant quantum-relaxation channel that, by driving the spins over Villain’s threshold, gives rise to fully-coherent, resonant spin tunneling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin-manipulation in graphene nanodevices. PMID:26641019

  18. Influences of Initial States on Entanglement Dynamics of Two Central Spins in a Spin Environment

    NASA Astrophysics Data System (ADS)

    Yu, Wen-Jian; Xu, Bao-Ming; Li, Lin; Zou, Jian; Li, Hai; Shao, Bin

    2016-03-01

    We investigate the entanglement dynamics of two electronic spins coupled to a bath of nuclear spins for two special cases, one is that two central spins both interact with a common bath, and the other is that one of two spins interacts with a bath. We consider three types of initial states with different correlations between the system and the bath, i.e., quantum correlation, classical correlation, and no-correlation. We show that the initial correlations (no matter quantum correlations or classical correlations) can effectively avoid the occurrence of entanglement sudden death. Irrespective of whether both two spins or only one of the two spins interacts with the bath, the system can gain more entanglement in the process of the time evolution for initial quantum correlations. In addition, we find that the effects of the distribution of coupling constants on entanglement dynamics crucially depend on the initial state of the spin bath.

  19. Low-Energy Spin Dynamics of the Honeycomb Spin Liquid Beyond the Kitaev Limit

    NASA Astrophysics Data System (ADS)

    Song, Xue-Yang; You, Yi-Zhuang; Balents, Leon

    2016-07-01

    We investigate the generic features of the low energy dynamical spin structure factor of the Kitaev honeycomb quantum spin liquid perturbed away from its exact soluble limit by generic symmetry-allowed exchange couplings. We find that the spin gap persists in the Kitaev-Heisenberg model, but generally vanishes provided more generic symmetry-allowed interactions exist. We formulate the generic expansion of the spin operator in terms of fractionalized Majorana fermion operators according to the symmetry enriched topological order of the Kitaev spin liquid, described by its projective symmetry group. The dynamical spin structure factor displays power-law scaling bounded by Dirac cones in the vicinity of the Γ , K , and K' points of the Brillouin zone, rather than the spin gap found for the exactly soluble point.

  20. Low-Energy Spin Dynamics of the Honeycomb Spin Liquid Beyond the Kitaev Limit.

    PubMed

    Song, Xue-Yang; You, Yi-Zhuang; Balents, Leon

    2016-07-15

    We investigate the generic features of the low energy dynamical spin structure factor of the Kitaev honeycomb quantum spin liquid perturbed away from its exact soluble limit by generic symmetry-allowed exchange couplings. We find that the spin gap persists in the Kitaev-Heisenberg model, but generally vanishes provided more generic symmetry-allowed interactions exist. We formulate the generic expansion of the spin operator in terms of fractionalized Majorana fermion operators according to the symmetry enriched topological order of the Kitaev spin liquid, described by its projective symmetry group. The dynamical spin structure factor displays power-law scaling bounded by Dirac cones in the vicinity of the Γ, K, and K^{'} points of the Brillouin zone, rather than the spin gap found for the exactly soluble point. PMID:27472139

  1. Static and dynamic elastic properties of rocks from the Canadian Shield

    SciTech Connect

    King, M.S.

    1983-01-01

    As part of a number of research studies in the Canadian Shield associated with the stability of underground mine openings, seismic reflection surveys, and the proposed use of a tunnel-boring machine (TBM) for developing mine headings, a long-term laboratory rock mechanics program has been conducted to determine the static and dynamic elastic properties of samples of igneous and metamorphic rocks from the Canadian Shield. This paper reports the results of 174 measurements of static elastic modulus and 152 measurements of uniaxial compressive strength for these rocks as a function of dynamic elastic modulus. 20 references, 5 figures.

  2. Dynamics of a macroscopic spin qubit in spin-orbit coupled Bose-Einstein condensates

    NASA Astrophysics Data System (ADS)

    Mardonov, Sh; Modugno, M.; Sherman, E. Ya

    2015-06-01

    We consider a macroscopic spin qubit based on spin-orbit coupled Bose-Einstein condensates, where, in addition to the spin-orbit coupling (SOC), spin dynamics strongly depends on the interaction between particles. The evolution of the spin for freely expanding, trapped, and externally driven condensates is investigated. For condensates oscillating at the frequency corresponding to the Zeeman splitting in the synthetic magnetic field, the spin Rabi frequency does not depend on the interaction between the atoms since it produces only internal forces and does not change the total momentum. However, interactions and SOC bring the system into a mixed spin state, where the total spin is inside rather than on the Bloch sphere. This greatly extends the available spin space making it three-dimensional, but imposes limitations on the reliable spin manipulation of such a macroscopic qubit. The spin dynamics can be modified by introducing suitable spin-dependent initial phases, determined by the SOC, in the spinor wave function.

  3. Sterically shielded spin labels for in-cell EPR spectroscopy: analysis of stability in reducing environment.

    PubMed

    Jagtap, A P; Krstic, I; Kunjir, N C; Hänsel, R; Prisner, T F; Sigurdsson, S Th

    2015-01-01

    Electron paramagnetic resonance (EPR) spectroscopy is a powerful and widely used technique for studying structure and dynamics of biomolecules under bio-orthogonal conditions. In-cell EPR is an emerging area in this field; however, it is hampered by the reducing environment present in cells, which reduces most nitroxide spin labels to their corresponding diamagnetic N-hydroxyl derivatives. To determine which radicals are best suited for in-cell EPR studies, we systematically studied the effects of substitution on radical stability using five different classes of radicals, specifically piperidine-, imidazolidine-, pyrrolidine-, and isoindoline-based nitroxides as well as the Finland trityl radical. Thermodynamic parameters of nitroxide reduction were determined by cyclic voltammetry; the rate of reduction in the presence of ascorbate, cellular extracts, and after injection into oocytes was measured by continuous-wave EPR spectroscopy. Our study revealed that tetraethyl-substituted nitroxides are good candidates for in-cell EPR studies, in particular pyrrolidine derivatives, which are slightly more stable than the trityl radical. PMID:25348344

  4. The Magnetic and Shielding Effects of Ring Current on Radiation Belt Dynamics

    NASA Technical Reports Server (NTRS)

    Fok, Mei-Ching

    2012-01-01

    The ring current plays many key roles in controlling magnetospheric dynamics. A well-known example is the magnetic depression produced by the ring current, which alters the drift paths of radiation belt electrons and may cause significant electron flux dropout. Little attention is paid to the ring current shielding effect on radiation belt dynamics. A recent simulation study that combines the Comprehensive Ring Current Model (CRCM) with the Radiation Belt Environment (RBE) model has revealed that the ring current-associated shielding field directly and/or indirectly weakens the relativistic electron flux increase during magnetic storms. In this talk, we will discuss how ring current magnetic field and electric shielding moderate the radiation belt enhancement.

  5. Controlling spin-spin network dynamics by repeated projective measurements

    PubMed Central

    Bretschneider, Christian O.; Álvarez, Gonzalo A.; Kurizki, Gershon; Frydman, Lucio

    2016-01-01

    We show that coupled-spin network manipulations can be made highly effective by repeated “projections” of the evolving quantum states onto diagonal density-matrix states (populations). As opposed to the intricately crafted pulse trains that are often used to fine-tune a complex network’s evolution, the strategy hereby presented derives from the “quantum-Zeno effect” and provides a highly robust route to guide the evolution by destroying all unwanted correlations (coherences). We exploit these effects by showing that a relaxation-like behaviour is endowed to polarization transfers occurring within a N-spin coupled network. Experimental implementations yield coupling constant determinations for complex spin-coupling topologies, as demonstrated within the field of liquid-state nuclear magnetic resonance (NMR). PMID:22540774

  6. Electron Spin Dynamics in Semiconductor Quantum Dots

    SciTech Connect

    Marie, X.; Belhadj, T.; Urbaszek, B.; Amand, T.; Krebs, O.; Lemaitre, A.; Voisin, P.

    2011-07-15

    An electron spin confined to a semiconductor quantum dot is not subject to the classical spin relaxation mechanisms known for free carriers but it strongly interacts with the nuclear spin system via the hyperfine interaction. We show in time resolved photoluminescence spectroscopy experiments on ensembles of self assembled InAs quantum dots in GaAs that this interaction leads to strong electron spin dephasing.

  7. Nonequilibrium dynamics of spin-orbit-coupled lattice bosons

    NASA Astrophysics Data System (ADS)

    Ng, H. T.

    2015-10-01

    We study the nonequilibrium dynamics of two-component bosonic atoms in a one-dimensional optical lattice in the presence of spin-orbit coupling. In the Mott-insulating regime, the two-component bosonic system at unity filling can be described by the quantum spin X X Z model. The atoms are initially prepared in their lower spin states. The system becomes out of equilibrium by suddenly introducing spin-orbit coupling to the atoms. The system shows the relaxation and nonstationary dynamics, respectively, in the different interaction regimes. We find that the time average of magnetization is useful to characterize the many-body dynamics. The effects of even and odd numbers of sites are discussed. Our result sheds light on nonequilibrium dynamics due to the interplay between spin-orbit coupling and atomic interactions.

  8. Nonlinear dynamics of spin and charge in spin-Calogero model

    SciTech Connect

    Kulkarni, Manas; Franchini, Fabio; Abanov, Alexander G.

    2009-10-15

    The fully nonlinear dynamics of spin and charge in spin-Calogero model is studied. The latter is an integrable one-dimensional model of quantum spin-1/2 particles interacting through inverse-square interaction and exchange. Classical hydrodynamic equations of motion are written for this model in the regime where gradient corrections to the exact hydrodynamic formulation of the theory may be neglected. In this approximation variables separate in terms of dressed Fermi momenta of the model. Hydrodynamic equations reduce to a set of decoupled Riemann-Hopf (or inviscid Burgers') equations for the dressed Fermi momenta. We study the dynamics of some nonequilibrium spin-charge configurations for times smaller than the time scale of the gradient catastrophe. We find an interesting interplay between spin and charge degrees of freedom. In the limit of large coupling constant the hydrodynamics reduces to the spin hydrodynamics of the Haldane-Shastry model.

  9. Semiclassical spin-spin dynamics and feedback control in transport through a quantum dot

    NASA Astrophysics Data System (ADS)

    Mosshammer, Klemens; Brandes, Tobias

    2014-10-01

    We present a theory of magnetotransport through an electronic orbital, where the electron spin interacts with a (sufficiently) large external spin via an exchange interaction. Using a semiclassical approximation, we derive a set of equations of motions for the electron density matrix and the mean value of the external spin that turns out to be highly nonlinear. The dissipation via the electronic leads is implemented in terms of a quantum master equation that is combined with the nonlinear terms of the spin-spin interaction. With an anisotropic exchange coupling a variety of dynamics is generated, such as self-sustained oscillations with parametric resonances or even chaotic behavior. Within our theory we can integrate a Maxwell-demon-like closed-loop feedback scheme that is capable of transporting particles against an applied bias voltage and that can be used to implement a spin filter to generate spin-dependent oscillating currents of opposite directions.

  10. Fractionation of plutonium in environmental and bio-shielding concrete samples using dynamic sequential extraction.

    PubMed

    Qiao, Jixin; Hou, Xiaolin

    2010-03-01

    Fractionation of plutonium isotopes ((238)Pu, (239,240)Pu) in environmental samples (i.e. soil and sediment) and bio-shielding concrete from decommissioning of nuclear reactor were carried out by dynamic sequential extraction using an on-line sequential injection (SI) system combined with a specially designed extraction column. Plutonium in the fractions from the sequential extraction was separated by ion exchange chromatography and measured using alpha spectrometry. The analytical results show a higher mobility of plutonium in bio-shielding concrete, which means attention should be paid to the treatment and disposal of nuclear waste from decommissioning. PMID:20004047

  11. Dynamics of test bodies with spin in de Sitter spacetime

    SciTech Connect

    Obukhov, Yuri N.; Puetzfeld, Dirk

    2011-02-15

    We study the motion of spinning test bodies in the de Sitter spacetime of constant positive curvature. With the help of the 10 Killing vectors, we derive the 4-momentum and the tensor of spin explicitly in terms of the spacetime coordinates. However, in order to find the actual trajectories, one needs to impose the so-called supplementary condition. We discuss the dynamics of spinning test bodies for the cases of the Frenkel and Tulczyjew conditions.

  12. Spin and charge dynamics of chromium alloys

    SciTech Connect

    Fishman, R.S.; Viswanath, V.S.; Liu, S.H.

    1996-07-01

    Both the spin- and charge-density waves of Cr alloys are produced by the Coulomb attraction between electrons and holes on nearly nested Fermi surfaces. Driven by quasi-particle transitions, transverse spin- wave and longitudinal phason modes are associated with rotational and translational symmetries of pure Cr and its dilute alloys. At low frequencies, both spin and charge phasons have a nearly linear dispersion with a mode velocity which approaches the spin-wave velocity as T approaches T{sub N} or as the mismatch between the Fermi surfaces increases.

  13. Understanding the Electronic Factors Responsible for Ligand Spin-Orbit NMR Shielding in Transition-Metal Complexes.

    PubMed

    Vícha, Jan; Foroutan-Nejad, Cina; Pawlak, Tomasz; Munzarová, Markéta L; Straka, Michal; Marek, Radek

    2015-04-14

    The significant role of relativistic effects in altering the NMR chemical shifts of light nuclei in heavy-element compounds has been recognized for a long time; however, full understanding of this phenomenon in relation to the electronic structure has not been achieved. In this study, the recently observed qualitative differences between the platinum and gold compounds in the magnitude and the sign of spin-orbit-induced (SO) nuclear magnetic shielding at the vicinal light atom ((13)C, (15)N), σ(SO)(LA), are explained by the contractions of 6s and 6p atomic orbitals in Au complexes, originating in the larger Au nuclear charge and stronger scalar relativistic effects in gold complexes. This leads to the chemical activation of metal 6s and 6p atomic orbitals in Au complexes and their larger participation in bonding with the ligand, which modulates the propagation of metal-induced SO effects on the NMR signal of the LA via the Spin-Orbit/Fermi Contact (SO/FC) mechanism. The magnitude of the σ(SO)(LA) in these square-planar complexes can be understood on the basis of a balance between various metal-based 5d → 5d* and 6p → 6p* orbital magnetic couplings. The large and positive σ(SO)(LA) in platinum complexes is dominated by the shielding platinum-based 5d → 5d* magnetic couplings, whereas small or negative σ(SO)(LA) in gold complexes is related to the deshielding contribution of the gold-based 6p → 6p* magnetic couplings. Further, it is demonstrated that σ(SO)(LA) correlates quantitatively with the extent of M-LA electron sharing that is the covalence of the M-LA bond (characterized by the QTAIM delocalization index, DI). The present findings will contribute to further understanding of the origin and propagation of the relativistic effects influencing the experimental NMR parameters in heavy-element systems.

  14. Toward Ultrafast Spin Dynamics in Low Dimensional Semiconductors

    NASA Astrophysics Data System (ADS)

    Chiu, Yi-Hsin

    Since the discovery of long spin relaxation times of itinerant electrons up to 100 nanoseconds and spin diffusion lengths over 100 mum in GaAs, extraordinary advances in semiconductor spintronics have been made in the past one and half decades. Incorporating spins in semiconductors requires the following essential capabilities: (i) injection of spins into semiconductors, (ii) manipulation of spins, and (iii) sensitive detection of spin coherence. The solutions to these challenges lie in a deeper understanding of spin interactions and spin relaxation in semiconductors as well as appropriate tools to probe spin dynamics. In particular, recent experiments have suggested the important role of dimensionality in spin dynamics. For example, spin-orbit interaction, the dominant source of spin relaxation in most II-VI and III-V semiconductors, has been shown to be significantly suppressed in reduced dimensions. Low-dimensional semiconductors are therefore appealing candidates for exploring spin physics and device applications. This dissertation aims at exploring spin dynamics in low dimensional semiconductor systems using time-resolved optical techniques. The time resolution allows for a direct measurement of the equilibrium and non-equilibrium carrier spins and various spin interactions in the time domain. Optical approaches are also a natural fit for probing optically active nanostructures where electric approaches can often encounter challenges. For instance, fabricating electric contacts with nanostructures is a proven challenge because of their reduced size and modified electronic structure. This dissertation is divided into three sections targeting an ultimate goal of employing optical methods to explore spin dynamics in low dimensional semiconductors. First, the time-resolved Kerr rotation technique is employed to study spin relaxation in Fe/MgO/GaAs heterostructures. The results reveal rich interactions between the GaAs electron spins, nuclear spins, and the

  15. Spin dynamics simulation of electron spin relaxation in Ni{sup 2+}(aq)

    SciTech Connect

    Rantaharju, Jyrki Mareš, Jiří Vaara, Juha

    2014-07-07

    The ability to quantitatively predict and analyze the rate of electron spin relaxation of open-shell systems is important for electron paramagnetic resonance and paramagnetic nuclear magnetic resonance spectroscopies. We present a combined molecular dynamics (MD), quantum chemistry (QC), and spin dynamics simulation method for calculating such spin relaxation rates. The method is based on the sampling of a MD trajectory by QC calculations, to produce instantaneous parameters of the spin Hamiltonian used, in turn, to numerically solve the Liouville-von Neumann equation for the time evolution of the spin density matrix. We demonstrate the approach by simulating the relaxation of electron spin in an aqueous solution of Ni{sup 2+} ion. The spin-lattice (T{sub 1}) and spin-spin (T{sub 2}) relaxation rates are extracted directly from the simulations of the time dependence of the longitudinal and transverse magnetization, respectively. Good agreement with the available, indirectly obtained experimental data is obtained by our method.

  16. Domain-wall spin dynamics in kagome antiferromagnets.

    PubMed

    Lhotel, E; Simonet, V; Ortloff, J; Canals, B; Paulsen, C; Suard, E; Hansen, T; Price, D J; Wood, P T; Powell, A K; Ballou, R

    2011-12-16

    We report magnetization and neutron scattering measurements down to 60 mK on a new family of Fe based kagome antiferromagnets, in which a strong local spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce unfamiliar slow spin dynamics in the ordered phase, evolving from exchange-released spin flips towards a cooperative behavior on decreasing the temperature, probably due to the onset of long-range dipolar interaction. A domain structure of independent magnetic grains is obtained that could be generic to other frustrated magnets.

  17. Dynamical properties of the hypercell spin-glass model

    NASA Astrophysics Data System (ADS)

    Gleiser, P. M.; Tamarit, F. A.

    1998-02-01

    The spreading of damage technique is used to study the dynamical phase diagram of the spin-glass hypercubic cell model in a heat bath Monte Carlo simulation. Since the hypercubic cell in dimension 2D and the hypercubic lattice in dimension D resemble each other closely at finite dimensions and both converge to a mean field when dimension goes to infinity, we can study the effects of dimensionality on the dynamical behavior of spin glasses.

  18. Cosmological dynamics with propagating Lorentz connection modes of spin zero

    SciTech Connect

    Chen, Hsin; Ho, Fei-Hung; Nester, James M.; Wang, Chih-Hung; Yo, Hwei-Jang E-mail: 93242010@cc.ncu.edu.tw E-mail: chwang@phy.ncu.edu.tw

    2009-10-01

    The Poincaré gauge theory of gravity has a Lorentz connection with both torsion and curvature. For this theory two good propagating connection modes, carrying spin-0{sup +} and spin-0{sup −}, have been found. The possible effects of the spin-0{sup +} mode in cosmology were investigated in a previous work by our group; there it was found that the 0{sup +} mode could account for the presently accelerating universe. Here, we extend the analysis to also include the spin-0{sup −} mode. The resulting cosmological model has three degrees of freedom. We present both the Lagrangian and Hamiltonian form of the dynamic equations for this model, find the late-time normal modes, and present some numerical evolution cases. In the late time asymptotic regime the two dynamic modes decouple, and the acceleration of the Universe oscillates due to the spin-0{sup +} mode.

  19. Gilbert damping of ferromagnetic metals incorporating inhomogeneous spin dynamics

    SciTech Connect

    Umetsu, Nobuyuki Miura, Daisuke; Sakuma, Akimasa

    2015-05-07

    The effects of inhomogeneous spin dynamics on magnetic damping in ferromagnetic metals are studied. On the basis of linear response theory, we derive the microscopic expression for the Gilbert damping term in a two-dimensional electron gas interacting with the magnetization via exchange coupling in the presence of Rashba spin-orbit coupling (SOC). In the spin wave propagating with the wave vector, q, the behavior of q-dependent damping can be explained in terms of both inter- and intra-band spin excitations. The spatially dependent damping torques originating from Rashba SOC that cancel out in a uniform precession system distort the circular orbit of a magnetization-precession trajectory in the presence of inhomogeneous spin dynamics.

  20. Dynamics, synchronization, and quantum phase transitions of two dissipative spins

    SciTech Connect

    Orth, Peter P.; Le Hur, Karyn; Roosen, David; Hofstetter, Walter

    2010-10-01

    We analyze the static and dynamic properties of two Ising-coupled quantum spins embedded in a common bosonic bath as an archetype of dissipative quantum mechanics. First, we elucidate the ground-state phase diagram for an Ohmic and a sub-Ohmic bath using a combination of bosonic numerical renormalization group (NRG), analytical techniques, and intuitive arguments. Second, by employing the time-dependent NRG we investigate the system's rich dynamical behavior arising from the complex interplay between spin-spin and spin-bath interactions. Interestingly, spin oscillations can synchronize due to the proximity of the common non-Markovian bath and the system displays highly entangled steady states for certain nonequilibrium initial preparations. We complement our nonperturbative numerical results by exact analytical solutions when available and provide quantitative limits on the applicability of the perturbative Bloch-Redfield approach at weak coupling.

  1. Spin motive force driven by skyrmion dynamics in magnetic nanodisks

    NASA Astrophysics Data System (ADS)

    Shimada, Yuhki; Ohe, Jun-ichiro

    2015-05-01

    The spin motive force driven by the dynamics of the skyrmion structure formed in a nanomagnetic disk is numerically investigated. Due to the existence of the magnetic structure along the disk edge, the collective mode of the magnetization is modified from that of the bulk skyrmion lattice obtained by using the periodic boundary condition. For a single-skyrmion disk, the dynamics of the skyrmion core and the edge magnetization induce the spin motive force, and a measurable AC voltage is obtained by two probes on the disk. For a multi-skyrmions disk, the phase-locked collective mode of skyrmions is found in the lowest resonant frequency where the amplitude of the AC voltage is enhanced by the cascade effect of the spin motive force. We also investigate the effect of the Rashba spin-orbit coupling on the spin motive force.

  2. NMR with generalized dynamics of spin and spatial coordinates

    SciTech Connect

    Lee, Chang Jae

    1987-11-01

    This work is concerned with theoretical and experimental aspects of the generalized dynamics of nuclear spin and spatial coordinates under magnetic-field pulses and mechanical motions. The main text begins with an introduction to the concept of ''fictitious'' interactions. A systematic method for constructing fictitious spin-1/2 operators is given. The interaction of spins with a quantized-field is described. The concept of the fictitious interactions under the irradiation of multiple pulses is utilized to design sequences for selectively averaging linear and bilinear operators. Relations between the low-field sequences and high-field iterative schemes are clarified. These relations and the transformation properties of the spin operators are exploited to develop schemes for heteronuclear decoupling of multi-level systems. The resulting schemes are evaluated for heteronuclear decoupling of a dilute spin-1/2 from a spin-1 in liquid crystal samples and from a homonuclear spin-1/2 pair in liquids. A relation between the spin and the spatial variables is discussed. The transformation properties of the spin operators are applied to spatial coordinates and utilized to develop methods for removing the orientational dependence responsible for line broadening in a powder sample. Elimination of the second order quadrupole effects, as well as the first order anisotropies is discussed. It is shown that various sources of line broadening can effectively be eliminated by spinning and/or hopping the sample about judiciously chosen axes along with appropriate radio-frequency pulse sequences.

  3. Spin supercurrent, magnetization dynamics, and φ-state in spin-textured Josephson junctions

    NASA Astrophysics Data System (ADS)

    Kulagina, Iryna; Linder, Jacob

    2014-08-01

    The prospect of combining the dissipationless nature of superconducting currents with the spin polarization of magnetic materials is interesting with respect to exploring superconducting analogs of topics in spintronics. In order to accomplish this aim, it is pivotal to understand not only how such spin supercurrents can be created, but also how they interact dynamically with magnetization textures. In this paper, we investigate the appearance of a spin supercurrent and the resulting magnetization dynamics in a textured magnetic Josephson current by using three experimentally relevant models: (i) a superconductor∣ferromagnet∣superconductor (S∣F∣S) junction with spin-active interfaces, (ii) a S∣F1∣F2∣F3∣S Josephson junction with a ferromagnetic trilayer, and (iii) a Josephson junction containing a domain wall. In all of these cases, the supercurrent is spin polarized and exerts a spin-transfer torque on the ferromagnetic interlayers which causes magnetization dynamics. Using a scattering matrix formalism in the clean limit, we compute the Andreev bound states and resulting free energy of the system which in turn is used to solve the Landau-Lifshiftz-Gilbert equation. We compute both how the inhomogeneous magnetism influences the phase dependence of the charge supercurrent and the magnetization dynamics caused by the spin polarization of the supercurrent. Using a realistic experimental parameter set, we find that the spin supercurrent can induce magnetization switching that is controlled by the superconducting phase difference. Moreover, we demonstrate that the combined effect of chiral spin symmetry breaking of the system as a whole with interface scattering causes the systems above to act as phase batteries that may supply any superconducting phase difference φ in the ground state. Such a φ-junction is accompanied by an anomalous supercurrent appearing even at zero phase difference, and we demonstrate that the flow direction of this current is

  4. Coherent Spin Dynamics in Semiconductor Nanostructures

    NASA Astrophysics Data System (ADS)

    Flatté, Michael E.

    2004-03-01

    Manipulation of coherent spins in semiconductors without laboratory AC (or in some cases DC) magnetic fields can be driven with the electronic spin-orbit interaction. This relativistic effect produces ``pseudomagnetic'' fields surpassing plausible laboratory magnetic fields by orders of magnitude. The theory of two principal examples will be described here: the coupling between light fields and electron spin in quantum dots, and the use of DC electric fields to manipulate spin coherence times in quantum wells. We find that intense coherent optical illumination of quantum dots can generate ultrafast ˜ 1000 Tesla pseudomagnetic fields suitable for electron spin rotation. These effective fields are roughly spherically symmetric for colloidal quantum dots, but for structurally aspherical quantum dots (such as self-assembled dots during molecular beam epitaxy growth) these pseudomagnetic fields are highly anisotropic - large parallel to the growth direction and often a factor of five or ten smaller along perpendicular directions. The structural anisotropy also leads to very anisotropic selection rules for light emission in quantum dot spin-light-emitting-diodes. For the second principal example, manipulation of spin coherence times in quantum wells, the zero-field spin coherence times and the tuning ranges depend strongly on the crystalline orientation of the growth axis. Near room temperature in (110)-grown structures for applied electric fields of 10-100 kV/cm, the tuning range can exceed several orders of magnitude. This work was done in collaboration with W. H. Lau and C. E. Pryor and was supported by DARPA/ARO and an ARO MURI.

  5. Nonadiabatic multichannel dynamics of a spin-orbit-coupled condensate

    NASA Astrophysics Data System (ADS)

    Xiong, Bo; Zheng, Jun-hui; Wang, Daw-wei

    2015-06-01

    We investigate the nonadiabatic dynamics of a driven spin-orbit-coupled Bose-Einstein condensate in both weak and strong driven force. It is shown that the standard Landau-Zener (LZ) tunneling fails in the regime of weak driven force and/or strong spin-orbital coupling, where the full nonadiabatic dynamics requires a new mechanism through multichannel effects. Beyond the semiclassical approach, our numerical and analytical results show an oscillating power-law decay in the quantum limit, different from the exponential decay in the semiclassical limit of the LZ effect. Furthermore, the condensate density profile is found to be dynamically fragmented by the multichannel effects and enhanced by interaction effects. Our work therefore provides a complete picture to understand the nonadiabatic dynamics of a spin-orbit coupled condensate, including various ranges of driven force and interaction effects through multichannel interference. The experimental indication of these nonadiabatic dynamics is also discussed.

  6. Simulating spin dynamics in organic solids under heteronuclear decoupling.

    PubMed

    Frantsuzov, Ilya; Ernst, Matthias; Brown, Steven P; Hodgkinson, Paul

    2015-09-01

    Although considerable progress has been made in simulating the dynamics of multiple coupled nuclear spins, predicting the evolution of nuclear magnetisation in the presence of radio-frequency decoupling remains challenging. We use exact numerical simulations of the spin dynamics under simultaneous magic-angle spinning and RF decoupling to determine the extent to which numerical simulations can be used to predict the experimental performance of heteronuclear decoupling for the CW, TPPM and XiX sequences, using the methylene group of glycine as a model system. The signal decay times are shown to be strongly dependent on the largest spin order simulated. Unexpectedly large differences are observed between the dynamics with and without spin echoes. Qualitative trends are well reproduced by modestly sized spin system simulations, and the effects of finite spin-system size can, in favourable cases, be mitigated by extrapolation. Quantitative prediction of the behaviour in complex parameter spaces is found, however, to be very challenging, suggesting that there are significant limits to the role of numerical simulations in RF decoupling problems, even when specialist techniques, such as state-space restriction, are used.

  7. The spin-temperature theory of dynamic nuclear polarization and nuclear spin-lattice relaxation

    NASA Technical Reports Server (NTRS)

    Byvik, C. E.; Wollan, D. S.

    1974-01-01

    A detailed derivation of the equations governing dynamic nuclear polarization (DNP) and nuclear spin lattice relaxation by use of the spin temperature theory has been carried to second order in a perturbation expansion of the density matrix. Nuclear spin diffusion in the rapid diffusion limit and the effects of the coupling of the electron dipole-dipole reservoir (EDDR) with the nuclear spins are incorporated. The complete expression for the dynamic nuclear polarization has been derived and then examined in detail for the limit of well resolved solid effect transitions. Exactly at the solid effect transition peaks, the conventional solid-effect DNP results are obtained, but with EDDR effects on the nuclear relaxation and DNP leakage factor included. Explicit EDDR contributions to DNP are discussed, and a new DNP effect is predicted.

  8. Incomplete fusion dynamics by spin distribution measurements

    SciTech Connect

    Singh, D.; Ali, R.; Ansari, M. Afzal; Singh, Pushpendra P.; Sharma, M. K.; Singh, B. P.; Babu, K. Surendra; Sinha, Rishi K.; Kumar, R.; Muralithar, S.; Singh, R. P.; Bhowmik, R. K.

    2010-02-15

    Spin distributions for various evaporation residues populated via complete and incomplete fusion of {sup 16}O with {sup 124}Sn at 6.3 MeV/nucleon have been measured, using charged particles (Z=1,2)-{gamma} coincidence technique. Experimentally measured spin distributions of the residues produced as incomplete fusion products associated with 'fast'{alpha}- and 2{alpha}-emission channels observed in the 'forward cone' are found to be distinctly different from those of the residues produced as complete fusion products. Moreover, 'fast'{alpha}-particles that arise from larger angular momentum in the entrance channel are populated at relatively higher driving input angular momentum than those produced through complete fusion. The incomplete fusion residues are populated in a limited, higher-angular-momentum range, in contrast to the complete fusion products, which are populated over a broad spin range.

  9. Enhancement of spin coherence in a spin-1 Bose-Einstein condensate by dynamical decoupling approaches

    SciTech Connect

    Ning Boyuan; Zhuang Jun; Zhang Wenxian; You, J. Q.

    2011-07-15

    We study the enhancement of spin coherence with periodic, concatenated, or Uhrig dynamical decoupling N-pulse sequences in a spin-1 Bose-Einstein condensate, where the intrinsic dynamical instability in such a ferromagnetically interacting condensate causes spin decoherence and eventually leads to a multiple spatial-domain structure or a spin texture. Our results show that all three sequences successfully enhance the spin coherence by pushing the wave vector of the most unstable mode in the condensate to a larger value. Among the three sequences with the same number of pulses, the concatenated one shows the best performance in preserving the spin coherence. More interestingly, we find that all three sequences exactly follow the same enhancement law, k{sub -}T{sup 1/2}=c, with k{sub -} the wave vector of the most unstable mode, T the sequence period, and c a sequence-dependent constant. Such a law between k{sub -} and T is also derived analytically for an attractive scalar Bose-Einstein condensate subjected to a periodic dynamical decoupling sequence.

  10. Fractional Spin Fluctuations as a Precursor of Quantum Spin Liquids: Majorana Dynamical Mean-Field Study for the Kitaev Model

    NASA Astrophysics Data System (ADS)

    Yoshitake, Junki; Nasu, Joji; Motome, Yukitoshi

    2016-10-01

    Experimental identification of quantum spin liquids remains a challenge, as the pristine nature is to be seen in asymptotically low temperatures. We here theoretically show that the precursor of quantum spin liquids appears in the spin dynamics in the paramagnetic state over a wide temperature range. Using the cluster dynamical mean-field theory and the continuous-time quantum Monte Carlo method, which are newly developed in the Majorana fermion representation, we calculate the dynamical spin structure factor, relaxation rate in nuclear magnetic resonance, and magnetic susceptibility for the honeycomb Kitaev model whose ground state is a canonical example of the quantum spin liquid. We find that dynamical spin correlations show peculiar temperature and frequency dependence even below the temperature where static correlations saturate. The results provide the experimentally accessible symptoms of the fluctuating fractionalized spins evincing the quantum spin liquids.

  11. Simulation of Spin-orbit Dynamics in Storage Rings

    NASA Astrophysics Data System (ADS)

    Ivanov, A.; Andrianov, S.; Senichev, Yu.

    2016-09-01

    In the article a mapping approach based on nonlinear matrix integration for longterm spin-orbit dynamics simulation is briefly described. Using this technique the nonlinear effects of spin dynamics in an electrostatics storage ring are investigated. Namely, the fringe fields, the energy conservation law and the random field errors are considered. The necessity of examination of such effects arises, for example, in the storage ring design for search the Electrical Dipole Moment of proton and deuteron. The EDM ring is proposed to measure EDM using the spin transformation of polarized particle in the magneto-electrostatic elements of the ring. The article consists of short description of the spin-orbit simulation results based on the nonlinear model.

  12. Numerical Researches on Dynamical Systems with Relativistic Spin

    NASA Astrophysics Data System (ADS)

    Han, W. B.

    2010-04-01

    It is well known that spinning compact binaries are one of the most important research objects in the universe. Especially, EMRIs (extreme mass ratio inspirals) involving stellar compact objects which orbit massive black holes, are considered to be primary sources of gravitational radiation (GW) which could be detected by the space-based interferometer LISA. GW signals from EMRIs can be used to test general relativity, measure the masses and spins of central black holes and study essential physics near horizons. Compared with the situation without spin, the complexity of extreme objects, most of which rotate very fast, is much higher. So the dynamics of EMRI systems are numerically and analytically studied. We focus on how the spin effects on the dynamics of these systems and the produced GW radiations. Firstly, an ideal model of spinning test particles around Kerr black hole is considered. For equatorial orbits, we present the correct expression of effective potential and analyze the stability of circular orbits. Especially, the gravitational binding energy and frame-dragging effect of extreme Kerr black hole are much bigger than those without spin. For general orbits, spin can monotonically enlarge orbital inclination and destroy the symmetry of orbits about equatorial plane. It is the most important that extreme spin can produce orbital chaos. By carefully investigating the relations between chaos and orbital parameters, we point out that chaos usually appears for orbits with small pericenter, big eccentricity and orbital inclination. It is emphasized that Poincaré section method is invalid to detect the chaos of spinning particles, and the way of systems toward chaos is the period-doubling bifurcation. Furthermore, we study how spins effect on GW radiations from spinning test particles orbiting Kerr black holes. It is found that spins can increase orbit eccentricity and then make h+ component be detected more easily. But for h× component, because spins change

  13. Number Fluctuation Dynamics of Atomic Spin Mixing inside a Condensate

    SciTech Connect

    Chang, Lee; Zhai, Q.; Lu Rong; You, L.

    2007-08-24

    We investigate the quantum dynamics of number fluctuations inside an atomic condensate during coherent spin mixing among internal states of the ground state hyperfine manifold, by quantizing the semiclassical nonrigid pendulum model in terms of the conjugate variable pair: the relative phase and the atom number. Our result provides a theoretical basis that resolves the resolution limit, or the effective ''shot-noise'' level, for counting atoms that is needed to clearly detect quantum correlation effects in spin mixing.

  14. Robust dynamical decoupling sequences for individual-nuclear-spin addressing

    NASA Astrophysics Data System (ADS)

    Casanova, J.; Wang, Z.-Y.; Haase, J. F.; Plenio, M. B.

    2015-10-01

    We propose the use of non-equally-spaced decoupling pulses for high-resolution selective addressing of nuclear spins by a quantum sensor. The analytical model of the basic operating principle is supplemented by detailed numerical studies that demonstrate the high degree of selectivity and the robustness against static and dynamic control-field errors of this scheme. We exemplify our protocol with a nitrogen-vacancy-center-based sensor to demonstrate that it enables the identification of individual nuclear spins that form part of a large spin ensemble.

  15. Optically induced dynamic nuclear spin polarisation in diamond

    NASA Astrophysics Data System (ADS)

    Scheuer, Jochen; Schwartz, Ilai; Chen, Qiong; Schulze-Sünninghausen, David; Carl, Patrick; Höfer, Peter; Retzker, Alexander; Sumiya, Hitoshi; Isoya, Junichi; Luy, Burkhard; Plenio, Martin B.; Naydenov, Boris; Jelezko, Fedor

    2016-01-01

    The sensitivity of magnetic resonance imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz et al 2011 Neoplasia 13 81). Nuclear spins associated with the 13C carbon isotope (nuclear spin I = 1/2) in diamond possess uniquely long spin lattice relaxation times (Reynhardt and High 2011 Prog. Nucl. Magn. Reson. Spectrosc. 38 37). If they are present in diamond nanocrystals, especially when strongly polarised, they form a promising contrast agent for MRI. Current schemes for achieving nuclear polarisation, however, require cryogenic temperatures. Here we demonstrate an efficient scheme that realises optically induced 13C nuclear spin hyperpolarisation in diamond at room temperature and low ambient magnetic field. Optical pumping of a nitrogen-vacancy centre creates a continuously renewable electron spin polarisation which can be transferred to surrounding 13C nuclear spins. Importantly for future applications we also realise polarisation protocols that are robust against an unknown misalignment between magnetic field and crystal axis.

  16. Ultrafast spin dynamics and switching via spin transfer torque in antiferromagnets with weak ferromagnetism

    NASA Astrophysics Data System (ADS)

    Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki

    2016-10-01

    The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse.

  17. Ultrafast spin dynamics and switching via spin transfer torque in antiferromagnets with weak ferromagnetism

    PubMed Central

    Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki

    2016-01-01

    The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse. PMID:27713522

  18. Storing entanglement of nuclear spins via Uhrig dynamical decoupling

    SciTech Connect

    Roy, Soumya Singha; Mahesh, T. S.; Agarwal, G. S.

    2011-06-15

    Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single-qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal order of the Uhrig sequence in which a singlet state can be stored at high correlation for about 30 seconds.

  19. Dynamics of magnetization in ferromagnet with spin-transfer torque

    NASA Astrophysics Data System (ADS)

    Li, Zai-Dong; He, Peng-Bin; Liu, Wu-Ming

    2014-11-01

    We review our recent works on dynamics of magnetization in ferromagnet with spin-transfer torque. Driven by constant spin-polarized current, the spin-transfer torque counteracts both the precession driven by the effective field and the Gilbert damping term different from the common understanding. When the spin current exceeds the critical value, the conjunctive action of Gilbert damping and spin-transfer torque leads naturally the novel screw-pitch effect characterized by the temporal oscillation of domain wall velocity and width. Driven by space- and time-dependent spin-polarized current and magnetic field, we expatiate the formation of domain wall velocity in ferromagnetic nanowire. We discuss the properties of dynamic magnetic soliton in uniaxial anisotropic ferromagnetic nanowire driven by spin-transfer torque, and analyze the modulation instability and dark soliton on the spin wave background, which shows the characteristic breather behavior of the soliton as it propagates along the ferromagnetic nanowire. With stronger breather character, we get the novel magnetic rogue wave and clarify its formation mechanism. The generation of magnetic rogue wave mainly arises from the accumulation of energy and magnons toward to its central part. We also observe that the spin-polarized current can control the exchange rate of magnons between the envelope soliton and the background, and the critical current condition is obtained analytically. At last, we have theoretically investigated the current-excited and frequency-adjusted ferromagnetic resonance in magnetic trilayers. A particular case of the perpendicular analyzer reveals that the ferromagnetic resonance curves, including the resonant location and the resonant linewidth, can be adjusted by changing the pinned magnetization direction and the direct current. Under the control of the current and external magnetic field, several magnetic states, such as quasi-parallel and quasi-antiparallel stable states, out

  20. Ultrafast spin dynamics in II-VI diluted magnetic semiconductors with spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Ungar, F.; Cygorek, M.; Tamborenea, P. I.; Axt, V. M.

    2015-05-01

    We study theoretically the ultrafast spin dynamics of II-VI diluted magnetic semiconductors in the presence of spin-orbit interaction. Our goal is to explore the interplay or competition between the exchange sd coupling and the spin-orbit interaction in both bulk and quantum-well systems. For bulk materials we concentrate on Zn1 -xMnxSe and take into account the Dresselhaus interaction, while for quantum wells we examine Hg1 -x -yMnxCdyTe systems with a strong Rashba coupling. Our calculations were performed with a recently developed formalism which incorporates electronic correlations beyond mean-field theory originating from the exchange sd coupling. For both bulk and quasi-two-dimensional systems we find that, by varying the system parameters within realistic ranges, either of the two interactions can be chosen to play a dominant role or they can compete on an equal footing with each other. The most notable effect of the spin-orbit interaction in both types of system is the appearance of strong oscillations where the exchange sd coupling by itself causes only an exponential decay of the mean electronic spin components. The mean-field approximation is also studied and an analytical interpretation is given as to why it shows a strong suppression of the spin-orbit-induced dephasing of the spin component parallel to the Mn magnetic field.

  1. Theoretical aspects of Magic Angle Spinning - Dynamic Nuclear Polarization.

    PubMed

    Mentink-Vigier, Frederic; Akbey, Ümit; Oschkinat, Hartmut; Vega, Shimon; Feintuch, Akiva

    2015-09-01

    Magic Angle Spinning (MAS) combined with Dynamic Nuclear Polarization (DNP) has been proven in recent years to be a very powerful method for increasing solid-state NMR signals. Since the advent of biradicals such as TOTAPOL to increase the nuclear polarization new classes of radicals, with larger molecular weight and/or different spin properties have been developed. These have led to unprecedented signal gain, with varying results for different experimental parameters, in particular the microwave irradiation strength, the static field, and the spinning frequency. Recently it has been demonstrated that sample spinning imposes DNP enhancement processes that differ from the active DNP mechanism in static samples as upon sample spinning the DNP enhancements are the results of energy level anticrossings occurring periodically during each rotor cycle. In this work we present experimental results with regards to the MAS frequency dependence of the DNP enhancement profiles of four nitroxide-based radicals at two different sets of temperature, 110 and 160K. In fact, different magnitudes of reduction in enhancement are observed with increasing spinning frequency. Our simulation code for calculating MAS-DNP powder enhancements of small model spin systems has been improved to extend our studies of the influence of the interaction and relaxation parameters on powder enhancements. To achieve a better understanding we simulated the spin dynamics of a single three-spin system {ea-eb-n} during its steady state rotor periods and used the Landau-Zener formula to characterize the influence of the different anti-crossings on the polarizations of the system and their necessary action for reaching steady state conditions together with spin relaxation processes. Based on these model calculations we demonstrate that the maximum steady state nuclear polarization cannot become larger than the maximum polarization difference between the two electrons during the steady state rotor cycle. This

  2. Theoretical aspects of Magic Angle Spinning - Dynamic Nuclear Polarization.

    PubMed

    Mentink-Vigier, Frederic; Akbey, Ümit; Oschkinat, Hartmut; Vega, Shimon; Feintuch, Akiva

    2015-09-01

    Magic Angle Spinning (MAS) combined with Dynamic Nuclear Polarization (DNP) has been proven in recent years to be a very powerful method for increasing solid-state NMR signals. Since the advent of biradicals such as TOTAPOL to increase the nuclear polarization new classes of radicals, with larger molecular weight and/or different spin properties have been developed. These have led to unprecedented signal gain, with varying results for different experimental parameters, in particular the microwave irradiation strength, the static field, and the spinning frequency. Recently it has been demonstrated that sample spinning imposes DNP enhancement processes that differ from the active DNP mechanism in static samples as upon sample spinning the DNP enhancements are the results of energy level anticrossings occurring periodically during each rotor cycle. In this work we present experimental results with regards to the MAS frequency dependence of the DNP enhancement profiles of four nitroxide-based radicals at two different sets of temperature, 110 and 160K. In fact, different magnitudes of reduction in enhancement are observed with increasing spinning frequency. Our simulation code for calculating MAS-DNP powder enhancements of small model spin systems has been improved to extend our studies of the influence of the interaction and relaxation parameters on powder enhancements. To achieve a better understanding we simulated the spin dynamics of a single three-spin system {ea-eb-n} during its steady state rotor periods and used the Landau-Zener formula to characterize the influence of the different anti-crossings on the polarizations of the system and their necessary action for reaching steady state conditions together with spin relaxation processes. Based on these model calculations we demonstrate that the maximum steady state nuclear polarization cannot become larger than the maximum polarization difference between the two electrons during the steady state rotor cycle. This

  3. Tunable nonequilibrium dynamics of field quenches in spin ice

    PubMed Central

    Mostame, Sarah; Castelnovo, Claudio; Moessner, Roderich; Sondhi, Shivaji L.

    2014-01-01

    We present nonequilibrium physics in spin ice as a unique setting that combines kinematic constraints, emergent topological defects, and magnetic long-range Coulomb interactions. In spin ice, magnetic frustration leads to highly degenerate yet locally constrained ground states. Together, they form a highly unusual magnetic state—a “Coulomb phase”—whose excitations are point-like defects—magnetic monopoles—in the absence of which effectively no dynamics is possible. Hence, when they are sparse at low temperature, dynamics becomes very sluggish. When quenching the system from a monopole-rich to a monopole-poor state, a wealth of dynamical phenomena occur, the exposition of which is the subject of this article. Most notably, we find reaction diffusion behavior, slow dynamics owing to kinematic constraints, as well as a regime corresponding to the deposition of interacting dimers on a honeycomb lattice. We also identify potential avenues for detecting the magnetic monopoles in a regime of slow-moving monopoles. The interest in this model system is further enhanced by its large degree of tunability and the ease of probing it in experiment: With varying magnetic fields at different temperatures, geometric properties—including even the effective dimensionality of the system—can be varied. By monitoring magnetization, spin correlations or zero-field NMR, the dynamical properties of the system can be extracted in considerable detail. This establishes spin ice as a laboratory of choice for the study of tunable, slow dynamics. PMID:24379372

  4. Destination state screening of active spaces in spin dynamics simulations

    NASA Astrophysics Data System (ADS)

    Krzystyniak, M.; Edwards, Luke J.; Kuprov, Ilya

    2011-06-01

    We propose a novel avenue for state space reduction in time domain Liouville space spin dynamics simulations, using detectability as a selection criterion - only those states that evolve into or affect other detectable states are kept in the simulation. This basis reduction procedure (referred to as destination state screening) is formally exact and can be applied on top of the existing state space restriction techniques. As demonstrated below, in many cases this results in further reduction of matrix dimension, leading to considerable acceleration of many spin dynamics simulation types. Destination state screening is implemented in the latest version of the Spinach library (http://spindynamics.org).

  5. Local spin dynamics with the electron electric dipole moment

    NASA Astrophysics Data System (ADS)

    Fukuda, Masahiro; Soga, Kota; Senami, Masato; Tachibana, Akitomo

    2016-01-01

    The local spin dynamics of the electron is studied from the viewpoint of the electric dipole moment (EDM) of the electron in the framework of the quantum field theory. The improvements of the computational accuracy of the effective electric field (Eeff) for the EDM and the understanding of spin precession are important for the experimental determination of the upper bound of the EDM. Calculations of Eeff in YbF (2Σ1 /2 ), BaF (2Σ1 /2 ), ThO (3Δ1 ), and HF+ (2Π1 /2 ) are performed on the basis of the restricted active space configuration interaction approach by using the four-component relativistic electronic structure calculation. The spin precession is also discussed from the viewpoint of local spin torque dynamics. We show that a contribution to the torque density for the spin is brought into by the EDM. Distributions of the local spin angular momentum density and torque densities induced by external fields in the above molecules are calculated and a property related with large Eeff is discussed.

  6. Electron spin dynamics and spin-lattice relaxation of trityl radicals in frozen solutions.

    PubMed

    Chen, Hanjiao; Maryasov, Alexander G; Rogozhnikova, Olga Yu; Trukhin, Dmitry V; Tormyshev, Victor M; Bowman, Michael K

    2016-09-28

    Electron spin-lattice relaxation of two trityl radicals, d24-OX063 and Finland trityl, were studied under conditions relevant to their use in dissolution dynamic nuclear polarization (DNP). The dependence of relaxation kinetics on temperature up to 100 K and on concentration up to 60 mM was obtained at X- and W-bands (0.35 and 3.5 Tesla, respectively). The relaxation is quite similar at both bands and for both trityl radicals. At concentrations typical for DNP, relaxation is mediated by excitation transfer and spin-diffusion to fast-relaxing centers identified as triads of trityl radicals that spontaneously form in the frozen samples. These centers relax by an Orbach-Aminov mechanism and determine the relaxation, saturation and electron spin dynamics during DNP. PMID:27560644

  7. Shapiro like steps reveals molecular nanomagnets’ spin dynamics

    SciTech Connect

    Abdollahipour, Babak; Abouie, Jahanfar Ebrahimi, Navid

    2015-09-15

    We present an accurate way to detect spin dynamics of a nutating molecular nanomagnet by inserting it in a tunnel Josephson junction and studying the current voltage (I-V) characteristic. The spin nutation of the molecular nanomagnet is generated by applying two circularly polarized magnetic fields. We demonstrate that modulation of the Josephson current by the nutation of the molecular nanomagnet’s spin appears as a stepwise structure like Shapiro steps in the I-V characteristic of the junction. Width and heights of these Shapiro-like steps are determined by two parameters of the spin nutation, frequency and amplitude of the nutation, which are simply tuned by the applied magnetic fields.

  8. Versatile approach to spin dynamics in correlated electron systems

    NASA Astrophysics Data System (ADS)

    Behrmann, Malte; Lichtenstein, Alexander I.; Katsnelson, Mikhail I.; Lechermann, Frank

    2016-10-01

    Time-dependent spin phenomena in condensed matter are most often either described in the weakly correlated limit of metallic Stoner-Slater-like magnetism via band theory or in the strongly correlated limit of Heisenberg-like interacting spins in an insulator. However, many experimental studies, e.g., of (de)magnetization processes, focus on itinerant local-moment materials, such as transition metals and various of their compounds. We here present a general theoretical framework that is capable of addressing correlated spin dynamics, also in the presence of a vanishing charge gap. A real-space implementation of the time-dependent rotational-invariant slave boson methodology allows us to treat nonequilibrium spins numerically fast and efficiently beyond linear response as well as beyond the band-theoretical or Heisenberg limit.

  9. Molecular dynamics, spin dynamics study of phonon-magnon interactions in BCC iron

    NASA Astrophysics Data System (ADS)

    Perera, Dilina; Landau, David P.; Stocks, G. Malcolm; Nicholson, Don; Eisenbach, Markus; Yin, Junqi

    2013-03-01

    By combining an atomistic many-body potential (Finnis-Sinclair) with a classical Heisenberg-like spin Hamiltonian, we perform combined molecular and spin dynamics simulations to investigate phonon-magnon interactions in BCC iron. The coupling between atomic and spin degrees of freedom is established via a distance dependent exchange interaction derived from first principles electronic structure calculations. Coupled equations of motion are integrated using a second order Suzuki-Trotter decomposition of the exponential time evolution operator. To investigate the effect of lattice vibrations on spin wave spectrum, we calculate spin-spin and density-density dynamic structure factors S(q, ω), and compare that to the results obtained from pure spin dynamics simulations performed on a rigid lattice. In the presence of lattice vibrations, we observe an additional peak in the longitudinal spin-spin dynamic structure factor which coincides with the peak position in density-density dynanmic structure factor. Research sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, ''Center for Defect Physics,'' an Energy Frontier Research Center

  10. Spin dynamics in a Curie-switch.

    PubMed

    Kravets, A F; Tovstolytkin, A I; Dzhezherya, Yu I; Polishchuk, D M; Kozak, I M; Korenivski, V

    2015-11-11

    Ferromagnetic resonance properties of F1/f/F2/AF multilayers, where weakly ferromagnetic spacer f is sandwiched between strongly ferromagnetic layers F1 and F2, with F1 being magnetically soft and F2-magnetically hard due to exchange pinning to antiferromagnetic layer AF, are investigated. Spacer-mediated exchange coupling is shown to strongly affect the resonance fields of both F1 and F2 layers. Our theoretical calculations as well as measurements show that the key magnetic parameters of the spacer, which govern the ferromagnetic resonance in F1/f/F2/AF, are the magnetic exchange length (Λ), effective saturation magnetization at T  =  0 (m0) and effective Curie temperature (T(C)(eff)). The values of these key parameters are deduced from the experimental data for multilayers with f  =  Ni(x)Cu(100-x), for the key ranges in the Ni-concentration (x = 54 ÷ 70 at. %) and spacer thickness (d = 3 ÷ 6 nm). The results obtained provide a deeper insight into thermally-controlled spin precession and switching in magnetic nanostructures, with potential applications in spin-based oscillators and memory devices.

  11. Spin Dynamics during Ultrafast Optical Demagnetization

    NASA Astrophysics Data System (ADS)

    Eisebitt, Stefan

    2015-03-01

    Magnetic order can be influenced on a sub-picosecund time scale via femtosecond optical pulses. In particular, demagnetization and switching can be triggered optically and while the applications e.g. for magnetic data storage are obvious, the underlying mechanisms are still under debate. We have investigated the contribution of electronic transport to optical demagnetization via pump-probe experiments at free-electron x-ray lasers. In ferromagnetic thin film multilayers with perpendicular anisotropy, optically excited electrons can move within a labyrinth domain network. Using x-ray magnetic circular dichroism (XMCD) as a contrast mechanism for small angle x-ray scattering to probe the local magnetization, we observe an ultrafast broadening of the domain walls, consistent with the existence of superdiffusive spin currents. Via pump-probe x-ray holographic imaging we obtain real space images of the local magnetization within the domain structure after pumping the system by a laterally confined excitation generated by an optical standing wave. With a temporal resolution of about 100 fs, we observe the propagation of a demagnetization front in real space, again consistent with the existence of superdiffusive spin currents. Support by BMBF in FSP-301 and 302 via Contracts 05K10KTB, 05K13KT3 and 05K13KT4 is gratefully acknowledged.

  12. Spin dynamics simulations for a nanoscale Heisenberg antiferromagnet

    NASA Astrophysics Data System (ADS)

    Hou, Zhuofei; Landau, D. P.; Brown, G.; Stocks, G. M.

    2010-03-01

    Thermoinduced magnetization(TiM) is a novel response which was predicted to occur in nanoscale antiferromagnetic materials. Extensive Monte Carlo simulations footnotetextG. Brown, A. Janotti, M. Eisenbach, and G. M. Stocks, Phys.Rev.B 72, 140405(2005) have shown that TiM is an intrinsic property of the antiferromagnetic classical Heisenberg model below the Neel temperature. To obtain a fundamental understanding of TiM, spin dynamics(SD) simulations are performed to study the spin wave behavior, which seems to be the cause of TiM. A classical Heisenberg model with an antiferromagnetic nearest-neighbor exchange interaction and uniaxial single-site anisotropy is studied. Simple-cubic lattices with free boundary conditions are used. We employed the fast spin dynamics algorithms with fourth-order Suzuki-Trotter decompositions of the exponential operator. Additional small excitation peaks due to surface effects are found in transverse S(q,w).

  13. Spin-Torque Driven Macrospin Dynamics subject to Thermal Noise

    NASA Astrophysics Data System (ADS)

    Pinna, Daniele

    This thesis considers the general Landau-Lifshitz-Gilbert theory underlying the magnetization dynamics of a macrospin subject to spin-torque effects and thermal fluctuations, as a function of the spin-polarization angle. The macrospin has biaxial magnetic anisotropy, typical of thin film magnetic elements, with an easy axis in the film plane and a hard axis out of the plane. When magnetic diffusion due to spin-torque and thermal noise effects occurs on a timescale that is much larger than the conservative precessional timescale due to magnetic anisotropies, it is possible to explore steady-state dynamics perturbatively by averaging the magnetization dynamics over constant energy orbits. This simplifies the magnetization dynamics to a 1D stochastic differential equation governing the evolution of the macropsin's energy. Current induced steady-state motions are then found to appear whenever the magnetization settles onto a stable constant energy trajectory where a balance of spin-torque and damping effects is achieved: with the remaining gyromagnetic motion due to anisotropy fields driving precessions. After averaging, all the relevant dynamical scenarios are found to depend on the ratio between hard and easy axis anisotropies. We derive the range of currents for which in-plane and out-of-plane limit cycles exist and discuss the regimes in which the constant energy orbit averaging technique is applicable. We find that there is a critical angle of the spin-polarization necessary for the occurrence of such states and predict a hysteretic response to applied current. This model can be tested in experiments on orthogonal spin-transfer devices, which consist of both an in-plane and out-of-plane magnetized spin-polarizers, effectively leading to an angle between the easy and spin-polarization axes. The technique developed allows for a detailed study of thermally driven macrospin escape phenomena within a stochastic Langevin framework. By employing Friedlin- Wentzell theory

  14. Terahertz electromagnons in spin-diluted cupric oxide: dynamics of twisted spin states

    NASA Astrophysics Data System (ADS)

    Lloyd-Hughes, James; Jones, Samuel; Wurz, Nicola; Failla, Michele; McConville, Chris; Prabhakaran, Dharmalingham

    2015-03-01

    Understanding the physics of magnetoelectric materials may lead to their application in actuators, sensors and solid state memories. Improper multiferroics also have novel quasiparticle excitations: electromagnons form when spin-waves become electric-dipole active. We investigated magnons, electromagnons and spin-lattice coupling in Cu(1-x)Zn(x)O (0dynamics was elucidated by Raman and Fourier-transform spectroscopy, showing strong spin-lattice coupling in Cu(1-x)Zn(x)O. While the phonon and magnon modes broaden and shift as a result of alloy-induced disorder, the electromagnon was found to be insensitive to Zn substitution and the induced disorder in the local spin structure. The results demonstrate that electromagnon excitations and dynamic magnetoelectric coupling can be maintained even in disordered spin systems, and at elevated temperatures.

  15. Magnetization dynamics of imprinted non-collinear spin textures

    SciTech Connect

    Streubel, Robert Kopte, Martin; Makarov, Denys; Fischer, Peter; Schmidt, Oliver G.

    2015-09-14

    We study the magnetization dynamics of non-collinear spin textures realized via imprint of the magnetic vortex state in soft permalloy into magnetically hard out-of-plane magnetized Co/Pd nanopatterned heterostructures. Tuning the interlayer exchange coupling between soft- and hard-magnetic subsystems provides means to tailor the magnetic state in the Co/Pd stack from being vortex- to donut-like with different core sizes. While the imprinted vortex spin texture leads to the dynamics similar to the one observed for vortices in permalloy disks, the donut-like state causes the appearance of two gyrofrequencies characteristic of the early and later stages of the magnetization dynamics. The dynamics are described using the Thiele equation supported by the full scale micromagnetic simulations by taking into account an enlarged core size of the donut states compared to magnetic vortices.

  16. Dynamical spin-density waves in a spin-orbit-coupled Bose-Einstein condensate

    NASA Astrophysics Data System (ADS)

    Li, Yan; Qu, Chunlei; Zhang, Yongsheng; Zhang, Chuanwei

    2015-07-01

    Synthetic spin-orbit (SO) coupling, an important ingredient for quantum simulation of many exotic condensed matter physics, has recently attracted considerable attention. The static and dynamic properties of a SO-coupled Bose-Einstein condensate (BEC) have been extensively studied in both theory and experiment. Here we numerically investigate the generation and propagation of a dynamical spin-density wave (SDW) in a SO-coupled BEC using a fast moving Gaussian-shaped barrier. We find that the SDW wavelength is sensitive to the barrier's velocity while varies slightly with the barrier's peak potential or width. We qualitatively explain the generation of SDW by considering a rectangular barrier in a one-dimensional system. Our results may motivate future experimental and theoretical investigations of rich dynamics in the SO-coupled BEC induced by a moving barrier.

  17. Absolute NMR shielding scales and nuclear spin-rotation constants in 175LuX and 197AuX (X = 19F, 35Cl, 79Br and 127I)

    NASA Astrophysics Data System (ADS)

    Demissie, Taye B.; Jaszuński, Michał; Komorovsky, Stanislav; Repisky, Michal; Ruud, Kenneth

    2015-10-01

    We present nuclear spin-rotation constants, absolute nuclear magnetic resonance (NMR) shielding constants, and shielding spans of all the nuclei in 175LuX and 197AuX (X = 19F, 35Cl, 79Br, 127I), calculated using coupled-cluster singles-and-doubles with a perturbative triples (CCSD(T)) correction theory, four-component relativistic density functional theory (relativistic DFT), and non-relativistic DFT. The total nuclear spin-rotation constants determined by adding the relativistic corrections obtained from DFT calculations to the CCSD(T) values are in general in agreement with available experimental data, indicating that the computational approach followed in this study allows us to predict reliable results for the unknown spin-rotation constants in these molecules. The total NMR absolute shielding constants are determined for all the nuclei following the same approach as that applied for the nuclear spin-rotation constants. In most of the molecules, relativistic effects significantly change the computed shielding constants, demonstrating that straightforward application of the non-relativistic formula relating the electronic contribution to the nuclear spin-rotation constants and the paramagnetic contribution to the shielding constants does not yield correct results. We also analyze the origin of the unusually large absolute shielding constant and its relativistic correction of gold in AuF compared to the other gold monohalides.

  18. Covariant hamiltonian spin dynamics in curved space-time

    NASA Astrophysics Data System (ADS)

    d'Ambrosi, G.; Satish Kumar, S.; van Holten, J. W.

    2015-04-01

    The dynamics of spinning particles in curved space-time is discussed, emphasizing the hamiltonian formulation. Different choices of hamiltonians allow for the description of different gravitating systems. We give full results for the simplest case with minimal hamiltonian, constructing constants of motion including spin. The analysis is illustrated by the example of motion in Schwarzschild space-time. We also discuss a non-minimal extension of the hamiltonian giving rise to a gravitational equivalent of the Stern-Gerlach force. We show that this extension respects a large class of known constants of motion for the minimal case.

  19. Computer studies of multiple-quantum spin dynamics

    SciTech Connect

    Murdoch, J.B.

    1982-11-01

    The excitation and detection of multiple-quantum (MQ) transitions in Fourier transform NMR spectroscopy is an interesting problem in the quantum mechanical dynamics of spin systems as well as an important new technique for investigation of molecular structure. In particular, multiple-quantum spectroscopy can be used to simplify overly complex spectra or to separate the various interactions between a nucleus and its environment. The emphasis of this work is on computer simulation of spin-system evolution to better relate theory and experiment.

  20. Dynamical scaling in Ising and vector spin glasses

    NASA Astrophysics Data System (ADS)

    Katzgraber, Helmut G.; Campbell, I. A.

    2005-07-01

    We have studied numerically the dynamics of spin glasses with Ising and XY symmetry (gauge glass) in space dimensions 2, 3, and 4. The nonequilibrium spin-glass susceptibility χne(tw,T) and the nonequilibrium energy per spin, ene(tw,T) , of samples of large size Lb are measured as a function of anneal time tw after a quench to temperatures T . The two observables are compared to the equilibrium spin-glass susceptibility χeq(L,T) and the equilibrium energy eeq(L,T) , respectively, measured as functions of temperature T and system size L for a range of system sizes. For any time and temperature a nonequilibrium time-dependent length scale L*(tw,T) can be defined by writing χne(tw,T)=χeq(L*,T) (or the equivalent expression for the energy). Our analysis shows that for all systems studied, an “effective dynamical critical exponent” parametrization L*(tw,T)=A(T)t1/z(T) fits the data well at each temperature within the whole temperature range studied, which extends from well above the critical temperature Tc to near T=0 for dimension 2 or to well below Tc for the other space dimensions studied. In addition, the data suggest that the dynamical exponent z varies smoothly when crossing the transition temperature.

  1. On the spin-axis dynamics of a Moonless Earth

    SciTech Connect

    Li, Gongjie; Batygin, Konstantin

    2014-07-20

    The variation of a planet's obliquity is influenced by the existence of satellites with a high mass ratio. For instance, Earth's obliquity is stabilized by the Moon and would undergo chaotic variations in the Moon's absence. In turn, such variations can lead to large-scale changes in the atmospheric circulation, rendering spin-axis dynamics a central issue for understanding climate. The relevant quantity for dynamically forced climate change is the rate of chaotic diffusion. Accordingly, here we re-examine the spin-axis evolution of a Moonless Earth within the context of a simplified perturbative framework. We present analytical estimates of the characteristic Lyapunov coefficient as well as the chaotic diffusion rate and demonstrate that even in absence of the Moon, the stochastic change in Earth's obliquity is sufficiently slow to not preclude long-term habitability. Our calculations are consistent with published numerical experiments and illustrate the putative system's underlying dynamical structure in a simple and intuitive manner.

  2. Spin-orbit ZORA and four-component Dirac-Coulomb estimation of relativistic corrections to isotropic nuclear shieldings and chemical shifts of noble gas dimers.

    PubMed

    Jankowska, Marzena; Kupka, Teobald; Stobiński, Leszek; Faber, Rasmus; Lacerda, Evanildo G; Sauer, Stephan P A

    2016-02-01

    Hartree-Fock and density functional theory with the hybrid B3LYP and general gradient KT2 exchange-correlation functionals were used for nonrelativistic and relativistic nuclear magnetic shielding calculations of helium, neon, argon, krypton, and xenon dimers and free atoms. Relativistic corrections were calculated with the scalar and spin-orbit zeroth-order regular approximation Hamiltonian in combination with the large Slater-type basis set QZ4P as well as with the four-component Dirac-Coulomb Hamiltonian using Dyall's acv4z basis sets. The relativistic corrections to the nuclear magnetic shieldings and chemical shifts are combined with nonrelativistic coupled cluster singles and doubles with noniterative triple excitations [CCSD(T)] calculations using the very large polarization-consistent basis sets aug-pcSseg-4 for He, Ne and Ar, aug-pcSseg-3 for Kr, and the AQZP basis set for Xe. For the dimers also, zero-point vibrational (ZPV) corrections are obtained at the CCSD(T) level with the same basis sets were added. Best estimates of the dimer chemical shifts are generated from these nuclear magnetic shieldings and the relative importance of electron correlation, ZPV, and relativistic corrections for the shieldings and chemical shifts is analyzed. PMID:26503739

  3. Matrix Formalism for Spin Dynamics Near a Single Depolarization Resonance

    SciTech Connect

    Chao, Alexander W.; /SLAC

    2005-10-26

    A matrix formalism is developed to describe the spin dynamics in a synchrotron near a single depolarization resonance as the particle energy (and therefore its spin precession frequency) is varied in a prescribed pattern as a function of time such as during acceleration. This formalism is first applied to the case of crossing the resonance with a constant crossing speed and a finite total step size, and then applied also to other more involved cases when the single resonance is crossed repeatedly in a prescribed manner consisting of linear ramping segments or sudden jumps. How repeated crossings produce an interference behavior is discussed using the results obtained. For a polarized beam with finite energy spread, a spin echo experiment is suggested to explore this interference effect.

  4. Dynamic-angle spinning and double rotation of quadrupolar nuclei

    SciTech Connect

    Mueller, K.T. California Univ., Berkeley, CA . Dept. of Chemistry)

    1991-07-01

    Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines causing crowding and overlap in NMR spectra. Magic- angle spinning, which is routinely used to produce high resolution spectra of spin-{1/2} nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids.

  5. Spacetime dynamics of spinning particles: Exact electromagnetic analogies

    NASA Astrophysics Data System (ADS)

    Costa, L. Filipe O.; Natário, José; Zilhão, Miguel

    2016-05-01

    We compare the rigorous equations describing the motion of spinning test particles in gravitational and electromagnetic fields, and show that if the Mathisson-Pirani spin condition holds then exact gravito-electromagnetic analogies emerge. These analogies provide a familiar formalism to treat gravitational problems, as well as a means for comparing the two interactions. Fundamental differences are manifest in the symmetries and time projections of the electromagnetic and gravitational tidal tensors. The physical consequences of the symmetries of the tidal tensors are explored comparing the following analogous setups: magnetic dipoles in the field of nonspinning/spinning charges, and gyroscopes in the Schwarzschild, Kerr, and Kerr-de Sitter spacetimes. The implications of the time projections of the tidal tensors are illustrated by the work done on the particle in various frames; in particular, a reciprocity is found to exist: in a frame comoving with the particle, the electromagnetic (but not the gravitational) field does work on it, causing a variation of its proper mass; conversely, for "static observers," a stationary gravitomagnetic (but not a magnetic) field does work on the particle, and the associated potential energy is seen to embody the Hawking-Wald spin-spin interaction energy. The issue of hidden momentum, and its counterintuitive dynamical implications, is also analyzed. Finally, a number of issues regarding the electromagnetic interaction and the physical meaning of Dixon's equations are clarified.

  6. Quantum spin dynamics in a spin-orbit-coupled Bose-Einstein condensate

    NASA Astrophysics Data System (ADS)

    Poon, Ting Fung Jeffrey; Liu, Xiong-Jun

    2016-06-01

    Spin-orbit-coupled bosons can exhibit rich equilibrium phases at low temperature and in the presence of particle-particle interactions. In the case with a 1D synthetic spin-orbit interaction, it has been observed that the ground state of a Bose gas can be a normal phase, stripe phase, or magnetized phase in different parameter regimes. The magnetized states are doubly degenerate and consist of a many-particle two-state system. In this work, we investigate the nonequilibrium quantum dynamics by switching on a simple one-dimensional optical lattice potential as external perturbation to induce resonant couplings between the magnetized phases, and predict a quantum spin dynamics which cannot be obtained in the single-particle systems. In particular, due to particle-particle interactions, the transition of the Bose condensate from one magnetized phase to the other is forbidden when the external perturbation strength is less than a critical value, and a full transition can occur only when the perturbation exceeds such critical strength. This phenomenon manifests itself a dynamical phase transition, with the order parameter defined by the time-averaged magnetization over an oscillation period, and the critical point behavior being exactly solvable. The thermal fluctuations are also considered in detail. From numerical simulations and exact analytic studies we show that the predicted many-body effects can be well observed with the current experiments.

  7. Current-driven spin dynamics in spin-orbit coupled superconductors

    NASA Astrophysics Data System (ADS)

    Vignale, Giovanni

    2012-02-01

    The study of the interplay between spin-orbit coupling (SOC) and superconductivity in two-dimensional electron gases (2DEG) has recently gained impetus following the discovery of i) 2DEGs in InAs or GaAs semiconductor heterostructures that are proximized by ordinary s-wave superconducting leads -- a class of systems which plays a key role in the quest for Majorana fermions -- and ii) 2DEGs that form at interfaces between complex oxides such as LaAlO3 and SrTiO3, which display tunable SOC and, under appropriate conditions, superconductivity. Motivated by this body of experimental and theoretical literature, we investigate the collective spin dynamics of an archetypical 2DEG model Hamiltonian with Rashba SOC in the presence of repulsive electron-electron (e-e) interactions. In the absence of superconductivity a Rashba 2DEG exhibits spin oscillations, which, at long wavelength and for weak repulsive interactions, have a frequency 2 αkF, α being the strength of SOC and kF the usual 2D Fermi wavenumber in the absence of SOC. These oscillations, however, are damped and quickly decay due to the emission of (double) electron-hole pairs, which, in the normal phase, are present at arbitrary low energies. In the presence of superconductivity, collective spin oscillations continue to exist in a wide range of parameters, because the Cooper pairs are mixtures of singlet and triplet components. Further, these excitations are undamped because they lie inside the superconducting gap where no other excitation exists. These spin oscillations can be excited by the application of a magnetic field or a supercurrent and can be used to realize persistent spin oscillators operating in the frequency range of 10 GHz - 1 THz.[4pt] Work supported by EU FP7 Programme Grant No. 215368-SEMISPINNET, No. 234970- NANOCTM and No. 248629-SOLID, and by NSF DMR-0705460.

  8. Dynamics of entanglement of two electron spins interacting with nuclear spin baths in quantum dots

    NASA Astrophysics Data System (ADS)

    Bragar, Igor; Cywiński, Łukasz

    2015-04-01

    We study the dynamics of entanglement of two electron spins in two quantum dots, in which each electron is interacting with its nuclear spin environment. Focusing on the case of uncoupled dots, and starting from either Bell or Werner states of two qubits, we calculate the decay of entanglement due to the hyperfine interaction with the nuclei. We mostly focus on the regime of magnetic fields in which the bath-induced electron spin flips play a role, for example, their presence leads to the appearance of entanglement sudden death at finite time for two qubits initialized in a Bell state. For these fields, the intrabath dipolar interactions and spatial inhomogeneity of hyperfine couplings are irrelevant on the time scale of coherence (and entanglement) decay, and most of the presented calculations are performed using the uniform-coupling approximation to the exact hyperfine Hamiltonian. We provide a comprehensive overview of entanglement decay in this regime, considering both free evolution of the qubits, and an echo protocol with simultaneous application of π pulses to the two spins. All the currently relevant for experiments bath states are considered: the thermal state, narrowed states (characterized by diminished uncertainty of one of the components of the Overhauser field) of two uncorrelated baths, and a correlated narrowed state with a well-defined value of the z component of the Overhauser field interdot gradient. While we mostly use concurrence to quantify the amount of entanglement in a mixed state of the two electron spins, we also show that their entanglement dynamics can be reconstructed from measurements of the currently relevant for experiments entanglement witnesses and the fidelity of quantum teleportation, performed using a partially disentangled state as a resource.

  9. Dynamical quantum phase transitions in random spin chains

    NASA Astrophysics Data System (ADS)

    Vosk, Ronen; Altman, Ehud

    2014-03-01

    Quantum systems can exhibit a great deal of universality at low temperature due to the structure of ground states and the critical points separating distinct states. On the other hand, quantum time evolution of the same systems involves all energies and it is therefore thought to be much harder, if at all possible, to have sharp transitions in the dynamics. In this paper we show that phase transitions characterized by universal singularities do occur in the time evolution of random spin chains. The sharpness of the transitions and integrity of the phases owes to many-body localization, which prevents thermalization in these systems. Using a renormalization group approach, we solve the time evolution of random Ising spin chains with generic interactions starting from initial states of arbitrary energy. As a function of the Hamiltonian parameters, the system is tuned through a dynamical transition, similar to the ground state critical point, at which the local spin correlations establish true long range temporal order. As in ground state quantum phase transitions, the dynamical transition has unique signatures in the entanglemenent properties of the system.

  10. Dynamics of hot random quantum spin chains: from anyons to Heisenberg spins

    NASA Astrophysics Data System (ADS)

    Parameswaran, Siddharth; Potter, Andrew; Vasseur, Romain

    2015-03-01

    We argue that the dynamics of the random-bond Heisenberg spin chain are ergodic at infinite temperature, in contrast to the many-body localized behavior seen in its random-field counterpart. First, we show that excited-state real-space renormalization group (RSRG-X) techniques suffer from a fatal breakdown of perturbation theory due to the proliferation of large effective spins that grow without bound. We repair this problem by deforming the SU (2) symmetry of the Heisenberg chain to its `anyonic' version, SU(2)k , where the growth of effective spins is truncated at spin S = k / 2 . This enables us to construct a self-consistent RSRG-X scheme that is particularly simple at infinite temperature. Solving the flow equations, we compute the excited-state entanglement and show that it crosses over from volume-law to logarithmic scaling at a length scale ξk ~eαk3 . This reveals that (a) anyon chains have random-singlet-like excited states for any finite k; and (b) ergodicity is restored in the Heisenberg limit k --> ∞ . We acknowledge support from the Quantum Materials program of LBNL (RV), the Gordon and Betty Moore Foundation (ACP), and UC Irvine startup funds (SAP).

  11. Second post-Newtonian Lagrangian dynamics of spinning compact binaries

    NASA Astrophysics Data System (ADS)

    Huang, Li; Wu, Xin; Ma, DaZhu

    2016-09-01

    The leading-order spin-orbit coupling is included in a post-Newtonian Lagrangian formulation of spinning compact binaries, which consists of the Newtonian term, first post-Newtonian (1PN) and 2PN non-spin terms and 2PN spin-spin coupling. This leads to a 3PN spin-spin coupling occurring in the derived Hamiltonian. The spin-spin couplings are mainly responsible for chaos in the Hamiltonians. However, the 3PN spin-spin Hamiltonian is small and has different signs, compared with the 2PN spin-spin Hamiltonian equivalent to the 2PN spin-spin Lagrangian. As a result, the probability of the occurrence of chaos in the Lagrangian formulation without the spin-orbit coupling is larger than that in the Lagrangian formulation with the spin-orbit coupling. Numerical evidences support this claim.

  12. Dynamics and stability of spinning flexible space tether systems

    NASA Astrophysics Data System (ADS)

    Tyc, George

    This dissertation focuses on a detailed dynamical investigation of a previously unexplored tether configuration that involves a spinning two-body tethered system with flexible appendages on each end-body where the spin axis is nominally aligned along the tether. The original motivation for this work came after the flight of the first Canadian sub-orbital tether mission OEDIPUS-A in 1989 which employed this spinning tethered configuration. To everyone's surprise, one of the end-bodies was observed to exhibit a rapid divergence of its nutation angle. It was clear after this flight that there were some fundamental mechanisms associated with the interaction between the tether and the end-body that were not fully understood at that time. Hence, a Tether Dynamics Experiment (TDE) was formed and became a formal part of the scientific agenda for the follow-on mission OEDIPUS-C which flew in 1995. This dissertation describes the work that was conducted as part of the TDE and involves: theoretical investigations into the dynamics of this spinning tethered flexible body system; ground testing to validate the models and establish the tether properties; application of the models to develop a stabilization approach for OEDIPUS-C, and comparisons between theory and flight data from both OEDIPUS-A and OEDIPUS-C. Nonlinear equations of motion are developed for a spinning tethered system where the tether could be either spinning with the end-bodies or attached to small de-spun platforms on the end-bodies. Since the tether used for the OEDIPUS missions is not a string, as is often assumed, but rather a wire that has some bending stiffness, albeit small, the tether bending was also taken into account in the formulation. Two sets of ground tests are described that were used to validate the stability conditions and gain confidence in the mathematical models. One set involved hanging a body by a tether and spinning at different speeds to investigate the end-body stability. The other set

  13. Dynamics of Rb and 21Ne spin ensembles interacting by spin exchange with a high Rb magnetic field

    NASA Astrophysics Data System (ADS)

    Fang, Jiancheng; Chen, Yao; Lu, Yan; Quan, Wei; Zou, Sheng

    2016-07-01

    We report on the dynamics of spin-polarized Rb and 21Ne ensembles in which the 21Ne spin ensemble in a glass vapor cell experiences a high magnetic field produced by a Rb electron-spin ensemble. The coupled spin ensembles are modeled and the response of the transverse-step magnetic field excitation is solved and studied experimentally. Moreover, we analyze the frequency response of the ensembles to a transverse-oscillating magnetic field. We demonstrate the strong transverse damping and large frequency shift of the 21Ne spin ensemble as the precession frequencies of 21Ne spin and Rb spin match and the magnetic resonance spectroscopies of the two ensembles merge into one. We also demonstrate the operation of the spin ensembles as a self-compensating co-magnetometer that is insensitive to low-frequency magnetic fields that would be useful for rotation rate sensing. For such sensing applications, a large Rb density is achieved to polarize the 21Ne spins. This density leads to a high Rb electron spin magnetic field and we demonstrate its effect on the dynamics of the co-magnetometer.

  14. precession: Dynamics of spinning black-hole binaries with python

    NASA Astrophysics Data System (ADS)

    Gerosa, Davide; Kesden, Michael

    2016-06-01

    We present the numerical code precession, a new open-source python module to study the dynamics of precessing black-hole binaries in the post-Newtonian regime. The code provides a comprehensive toolbox to (i) study the evolution of the black-hole spins along their precession cycles, (ii) perform gravitational-wave-driven binary inspirals using both orbit-averaged and precession-averaged integrations, and (iii) predict the properties of the merger remnant through fitting formulas obtained from numerical-relativity simulations. precession is a ready-to-use tool to add the black-hole spin dynamics to larger-scale numerical studies such as gravitational-wave parameter estimation codes, population synthesis models to predict gravitational-wave event rates, galaxy merger trees and cosmological simulations of structure formation. precession provides fast and reliable integration methods to propagate statistical samples of black-hole binaries from/to large separations where they form to/from small separations where they become detectable, thus linking gravitational-wave observations of spinning black-hole binaries to their astrophysical formation history. The code is also a useful tool to compute initial parameters for numerical-relativity simulations targeting specific precessing systems. precession can be installed from the python Package Index, and it is freely distributed under version control on github, where further documentation is provided.

  15. Dynamical Quantum Phase Transitions in Random Spin Chains

    NASA Astrophysics Data System (ADS)

    Vosk, Ronen; Altman, Ehud

    2014-05-01

    Using a renormalization group approach, we solve the time evolution of random Ising spin chains with generic interactions starting from initial states of arbitrary energy. As a function of the Hamiltonian parameters, the system is tuned through a dynamical transition, similar to the ground-state critical point, at which the local spin correlations establish true long-range temporal order. In the state with a dominant transverse field, a spin that starts in an up state loses its orientation with time, while in the "ordered" state it never does. As in ground-state quantum phase transitions, the dynamical transition has unique signatures in the entanglement properties of the system. When the system is initialized in a product state, the entanglement entropy grows as log(t) in the two "phases," while at the critical point it grows as logα(t), with α a universal number. This universal entanglement growth requires generic ("integrability breaking") interactions to be added to the pure transverse field Ising model.

  16. Planar spin-transfer device with dynamical polarizer and analizer

    NASA Astrophysics Data System (ADS)

    Bazaliy, Yaroslaw; Kravchenko, Anton

    2011-03-01

    The behavior of the planar spin-transfer devices with monodomain magnetic layers can be described by the macrospin Landau-Lifshitz-Gilbert (LLG) equation with spin-transfer terms. The LLG description of a device with two layers is simplified after applying the overdamped, large easy-plane anisotropy approximation. A decrease of the magnetic layer thickness asymmetry creates a transition from the conventional polarizer-analizer (``fixed layer -- free layer'') operation regime to the regime of the nearly identical magnets. Here electric current leads to a ``Slonczewski windmill'' dynamic state, rather than producing the magnetic switching. The ``windmill'' precession state of a device with two free layers was investigated by numerical solution of the LLG equation.

  17. Dynamic response of an artificial square spin ice

    NASA Astrophysics Data System (ADS)

    Jungfleisch, M. B.; Zhang, W.; Iacocca, E.; Sklenar, J.; Ding, J.; Jiang, W.; Zhang, S.; Pearson, J. E.; Novosad, V.; Ketterson, J. B.; Heinonen, O.; Hoffmann, A.

    2016-03-01

    Magnetization dynamics in an artificial square spin-ice lattice made of Ni80Fe20 with magnetic field applied in the lattice plane is investigated by broadband ferromagnetic resonance spectroscopy. The experimentally observed dispersion shows a rich spectrum of modes corresponding to different magnetization states. These magnetization states are determined by exchange and dipolar interaction between individual islands, as is confirmed by a semianalytical model. In the low field regime below 400 Oe a hysteretic behavior in the mode spectrum is found. Micromagnetic simulations reveal that the origin of the observed spectra is due to the initialization of different magnetization states of individual nanomagnets. Our results indicate that it might be possible to determine the spin-ice state by resonance experiments and are a first step towards the understanding of artificial geometrically frustrated magnetic systems in the high-frequency regime.

  18. Phase ordering dynamics in spin-1 ferromagnetic condensates

    NASA Astrophysics Data System (ADS)

    Williamson, Lewis; Blakie, Peter

    2016-05-01

    Spinor Bose-Einstein condensates present rich phase diagrams for exploring phase transitions between states with different symmetry properties. In this work we simulate the approach to equilibrium of a spin-1 condensate quenched from an unmagnetised phase to three different ferromagnetic phases. The three ferromagnetic phases have Z2, SO(2) and SO(3) symmetries respectively and possess different conservation laws. Following the quench, domains of magnetization form, with each domain making an independent choice of the symmetry breaking order parameter. These domains grow and compete for the global equilibrium state. We find that this growth follows universal scaling laws and identify the dynamic universality class for each of the three quenches. Polar-core spin-vortices play a crucial role in the phase ordering of the SO(2) system and we identify fractal structures in the domain patterns of the SO(2) and SO(3) systems. We acknowledge support from the Marsden Fund of New Zealand.

  19. Spin-density correlations in the dynamic spin-fluctuation theory: Comparison with polarized neutron scattering experiments

    NASA Astrophysics Data System (ADS)

    Melnikov, N. B.; Reser, B. I.; Paradezhenko, G. V.

    2016-08-01

    To study the spin-density correlations in the ferromagnetic metals above the Curie temperature, we relate the spin correlator and neutron scattering cross-section. In the dynamic spin-fluctuation theory, we obtain explicit expressions for the effective and local magnetic moments and spatial spin-density correlator. Our theoretical results are demonstrated by the example of bcc Fe. The effective and local moments are found in good agreement with results of polarized neutron scattering experiment over a wide temperature range. The calculated short-range order is small (up to 4 Å) and slowly decreases with temperature.

  20. Probing the dynamics of a nuclear spin bath in diamond through time-resolved central spin magnetometry.

    PubMed

    Dréau, A; Jamonneau, P; Gazzano, O; Kosen, S; Roch, J-F; Maze, J R; Jacques, V

    2014-09-26

    Using fast electron spin resonance spectroscopy of a single nitrogen-vacancy defect in diamond, we demonstrate real-time readout of the Overhauser field produced by its nuclear spin environment under ambient conditions. These measurements enable narrowing the Overhauser field distribution by postselection, corresponding to a conditional preparation of the nuclear spin bath. Correlations of the Overhauser field fluctuations are quantitatively inferred by analyzing the Allan deviation over consecutive measurements. This method allows us to extract the dynamics of weakly coupled nuclear spins of the reservoir.

  1. Probing the Dynamics of a Nuclear Spin Bath in Diamond through Time-Resolved Central Spin Magnetometry

    NASA Astrophysics Data System (ADS)

    Dréau, A.; Jamonneau, P.; Gazzano, O.; Kosen, S.; Roch, J.-F.; Maze, J. R.; Jacques, V.

    2014-09-01

    Using fast electron spin resonance spectroscopy of a single nitrogen-vacancy defect in diamond, we demonstrate real-time readout of the Overhauser field produced by its nuclear spin environment under ambient conditions. These measurements enable narrowing the Overhauser field distribution by postselection, corresponding to a conditional preparation of the nuclear spin bath. Correlations of the Overhauser field fluctuations are quantitatively inferred by analyzing the Allan deviation over consecutive measurements. This method allows us to extract the dynamics of weakly coupled nuclear spins of the reservoir.

  2. Effect of electron spin dynamics on solid-state dynamic nuclear polarization performance.

    PubMed

    Siaw, Ting Ann; Fehr, Matthias; Lund, Alicia; Latimer, Allegra; Walker, Shamon A; Edwards, Devin T; Han, Song-I

    2014-09-21

    For the broadest dissemination of solid-state dynamic nuclear polarization (ssDNP) enhanced NMR as a material characterization tool, the ability to employ generic mono-nitroxide radicals as spin probes is critical. A better understanding of the factors contributing to ssDNP efficiency is needed to rationally optimize the experimental condition for the practically accessible spin probes at hand. This study seeks to advance the mechanistic understanding of ssDNP by examining the effect of electron spin dynamics on ssDNP performance at liquid helium temperatures (4-40 K). The key observation is that bi-radicals and mono-radicals can generate comparable nuclear spin polarization at 4 K and 7 T, which is in contrast to the observation for ssDNP at liquid nitrogen temperatures (80-150 K) that finds bi-radicals to clearly outperform mono-radicals. To rationalize this observation, we analyze the change in the DNP-induced nuclear spin polarization (Pn) and the characteristic ssDNP signal buildup time as a function of electron spin relaxation rates that are modulated by the mono- and bi-radical spin concentration. Changes in Pn are consistent with a systematic variation in the product of the electron spin-lattice relaxation time and the electron spin flip-flop rate that constitutes an integral saturation factor of an inhomogeneously broadened EPR spectrum. We show that the comparable Pn achieved with both radical species can be reconciled with a comparable integral EPR saturation factor. Surprisingly, the largest Pn is observed at an intermediate spin concentration for both mono- and bi-radicals. At the highest radical concentration, the stronger inter-electron spin dipolar coupling favors ssDNP, while oversaturation diminishes Pn, as experimentally verified by the observation of a maximum Pn at an intermediate, not the maximum, microwave (μw) power. At the maximum μw power, oversaturation reduces the electron spin population differential that must be upheld between

  3. Spin-state configuration induced faster spin dynamics in epitaxial La1-xSrxCoO3 thin films

    NASA Astrophysics Data System (ADS)

    Cui, W. Y.; Li, P.; Bai, H. L.

    2015-05-01

    Two important features: spin-state configuration and spin dynamics in phase-separated ferromagnetic/spin-glass epitaxial La1-xSrxCoO3 thin films (x=0.07, 0.17, 0.26, 0.30, 0.40, 0.60) have been investigated and elaborated, proved by both magnetic analyses and first principle calculations. The configuration with high-spin (HS) state Co3+ and low-spin (LS) state Co4+ is considered to be the most stable spin-state configuration for La1-xSrxCoO3 at ground state, which was demonstrated by calculating the magnetic moments of La1-xSrxCoO3, as well as first principle calculation. The stretched Co-O bond by Sr doping causes the decrease of crystal field splitting, resulting in the HS state Co3+ and LS state Co4+. The spin dynamics in the La1-xSrxCoO3 thin films was found to be faster than the classic spin-glass compounds, which is attributed to the higher-spin Co3+, and rather smaller ferromagnetic cluster size (~2.16 to ~21.5 nm) in the epitaxial films than that in referenced polycrystalline compounds (~35 to ~240 nm).

  4. Random walk approach to spin dynamics in a two-dimensional electron gas with spin-orbit coupling

    SciTech Connect

    Yang, Luyi; Orenstein, J.; Lee, Dung-Hai

    2010-09-27

    We introduce and solve a semiclassical random walk (RW) model that describes the dynamics of spin polarization waves in zinc-blende semiconductor quantum wells. We derive the dispersion relations for these waves, including the Rashba, linear and cubic Dresselhaus spin-orbit interactions, as well as the effects of an electric field applied parallel to the spin polarization wave vector. In agreement with calculations based on quantum kinetic theory [P. Kleinert and V. V. Bryksin, Phys. Rev. B 76, 205326 (2007)], the RW approach predicts that spin waves acquire a phase velocity in the presence of the field that crosses zero at a nonzero wave vector, q{sub 0}. In addition, we show that the spin-wave decay rate is independent of field at q{sub 0} but increases as (q-q{sub 0}){sup 2} for q {ne} q{sub 0}. These predictions can be tested experimentally by suitable transient spin grating experiments.

  5. Spin dynamics and relaxation in the classical-spin Kondo-impurity model beyond the Landau-Lifschitz-Gilbert equation

    NASA Astrophysics Data System (ADS)

    Sayad, Mohammad; Potthoff, Michael

    2015-11-01

    The real-time dynamics of a classical spin in an external magnetic field and local exchange coupled to an extended one-dimensional system of non-interacting conduction electrons is studied numerically. Retardation effects in the coupled electron-spin dynamics are shown to be the source for the relaxation of the spin in the magnetic field. Total energy and spin is conserved in the non-adiabatic process. Approaching the new local ground state is therefore accompanied by the emission of dispersive wave packets of excitations carrying energy and spin and propagating through the lattice with Fermi velocity. While the spin dynamics in the regime of strong exchange coupling J is rather complex and governed by an emergent new time scale, the motion of the spin for weak J is regular and qualitatively well described by the Landau-Lifschitz-Gilbert (LLG) equation. Quantitatively, however, the full quantum-classical hybrid dynamics differs from the LLG approach. This is understood as a breakdown of weak-coupling perturbation theory in J in the course of time. Furthermore, it is shown that the concept of the Gilbert damping parameter is ill-defined for the case of a one-dimensional system.

  6. Spin and Beam Dynamics in the Muon (g - 2) Experiments

    NASA Astrophysics Data System (ADS)

    Semertzidis, Yannis K.

    2016-09-01

    A number of recent advances in the Physics of the Muon (g - 2) experiments are described outlining the expectations of future improvements of the statistical and systematic errors of the technique. A comparison between the spin and beam dynamics of the two muon (g - 2) experiments under preparation at FNAL and at J-PARC shows that they are both well under control. It may be possible to use magnetic focusing for the FNAL experiment, especially if a decision is made to run with negative muons. Finally, a polarized proton beam could be used to measure the B-field in case of magnetic focusing.

  7. Spin-down Dynamics of Magnetized Solar-type Stars

    NASA Astrophysics Data System (ADS)

    Oglethorpe, R. L. F.; Garaud, P.

    2013-12-01

    It has long been known that solar-type stars undergo significant spin-down, via magnetic braking, during their main-sequence lifetimes. However, magnetic braking only operates on the surface layers; it is not yet completely understood how angular momentum is transported within the star and how rapidly the spin-down information is communicated to the deep interior. In this work, we use insight from recent progress in understanding internal solar dynamics to model the interior of other solar-type stars. We assume, following Gough & McIntyre, that the bulk of the radiation zone of these stars is held in uniform rotation by the presence of an embedded large-scale primordial field, confined below a stably stratified, magnetic-free tachocline by large-scale meridional flows downwelling from the convection zone. We derive simple equations to describe the response of this model interior to spin-down of the surface layers, which are identical to the two-zone model of MacGregor & Brenner, with a coupling timescale proportional to the local Eddington-Sweet timescale across the tachocline. This timescale depends both on the rotation rate of the star and on the thickness of the tachocline, and it can vary from a few hundred thousand years to a few Gyr, depending on stellar properties. Qualitative predictions of the model appear to be consistent with observations, although they depend sensitively on the assumed functional dependence of the tachocline thickness on the stellar rotation rate.

  8. Spin-down dynamics of magnetized solar-type stars

    SciTech Connect

    Oglethorpe, R. L. F.; Garaud, P.

    2013-12-01

    It has long been known that solar-type stars undergo significant spin-down, via magnetic braking, during their main-sequence lifetimes. However, magnetic braking only operates on the surface layers; it is not yet completely understood how angular momentum is transported within the star and how rapidly the spin-down information is communicated to the deep interior. In this work, we use insight from recent progress in understanding internal solar dynamics to model the interior of other solar-type stars. We assume, following Gough and McIntyre, that the bulk of the radiation zone of these stars is held in uniform rotation by the presence of an embedded large-scale primordial field, confined below a stably stratified, magnetic-free tachocline by large-scale meridional flows downwelling from the convection zone. We derive simple equations to describe the response of this model interior to spin-down of the surface layers, which are identical to the two-zone model of MacGregor and Brenner, with a coupling timescale proportional to the local Eddington-Sweet timescale across the tachocline. This timescale depends both on the rotation rate of the star and on the thickness of the tachocline, and it can vary from a few hundred thousand years to a few Gyr, depending on stellar properties. Qualitative predictions of the model appear to be consistent with observations, although they depend sensitively on the assumed functional dependence of the tachocline thickness on the stellar rotation rate.

  9. Spin glass model for dynamics of cell reprogramming

    NASA Astrophysics Data System (ADS)

    Pusuluri, Sai Teja; Lang, Alex H.; Mehta, Pankaj; Castillo, Horacio E.

    2015-03-01

    Recent experiments show that differentiated cells can be reprogrammed to become pluripotent stem cells. The possible cell fates can be modeled as attractors in a dynamical system, the ``epigenetic landscape.'' Both cellular differentiation and reprogramming can be described in the landscape picture as motion from one attractor to another attractor. We perform Monte Carlo simulations in a simple model of the landscape. This model is based on spin glass theory and it can be used to construct a simulated epigenetic landscape starting from the experimental genomic data. We re-analyse data from several cell reprogramming experiments and compare with our simulation results. We find that the model can reproduce some of the main features of the dynamics of cell reprogramming.

  10. Spin-Polarized Nonadiabatic Dynamics with Local Basis Sets

    NASA Astrophysics Data System (ADS)

    Hoyt, Robert; Kolesov, Grigory; Tritsaris, Georgios; Granas, Oscar; Efthimios, Efthimios

    Accurate simulations of electron transfer at the solid-electrolyte interphase (SEI) are critical for understanding and predicting electrochemical reactions. Density-Functional Theory (DFT) has been widely applied to study the ground-state structure of novel materials for electrochemical energy storage and for adiabatic molecular dynamics. Unfortunately, many chemical reactions take place on femtosecond time scales where assuming adiabatic electron density propagation is invalid. To resolve this, we have developed the ability to perform time-dependent DFT calculations using nonadiabatic propagation of the electron density along with Ehrenfest dynamics for the ions to better capture the complex interactions that occur during surface-electrolyte electron transfer and chemical reactions. Spin polarization is also implemented to improve the accuracy of the simulations and their suitability for studying a wider range of chemical reactions. Local basis sets are implemented via linear combinations of atomic orbitals to reduce the size of the DFT basis for computational efficiency.

  11. Information-flux approach to multiple-spin dynamics

    NASA Astrophysics Data System (ADS)

    di Franco, C.; Paternostro, M.; Palma, G. M.; Kim, M. S.

    2007-10-01

    We introduce and formalize the concept of information flux in a many-body register as the influence that the dynamics of a specific element receive from any other element of the register. By quantifying the information flux in a protocol, we can design the most appropriate initial state of the system and, noticeably, the distribution of coupling strengths among the parts of the register itself. The intuitive nature of this tool and its flexibility, which allow for easily manageable numerical approaches when analytic expressions are not straightforward, are greatly useful in interacting many-body systems such as quantum spin chains. We illustrate the use of this concept in quantum cloning and quantum state transfer and we also sketch its extension to nonunitary dynamics.

  12. Information-flux approach to multiple-spin dynamics

    SciTech Connect

    Di Franco, C.; Paternostro, M.; Kim, M. S.; Palma, G. M.

    2007-10-15

    We introduce and formalize the concept of information flux in a many-body register as the influence that the dynamics of a specific element receive from any other element of the register. By quantifying the information flux in a protocol, we can design the most appropriate initial state of the system and, noticeably, the distribution of coupling strengths among the parts of the register itself. The intuitive nature of this tool and its flexibility, which allow for easily manageable numerical approaches when analytic expressions are not straightforward, are greatly useful in interacting many-body systems such as quantum spin chains. We illustrate the use of this concept in quantum cloning and quantum state transfer and we also sketch its extension to nonunitary dynamics.

  13. Dynamical spin structure factor of one-dimensional interacting fermions

    NASA Astrophysics Data System (ADS)

    Zyuzin, Vladimir A.; Maslov, Dmitrii L.

    2015-02-01

    We revisit the dynamic spin susceptibility χ (q ,ω ) of one-dimensional interacting fermions. To second order in the interaction, backscattering results in a logarithmic correction to χ (q ,ω ) at q ≪kF , even if the single-particle spectrum is linearized near the Fermi points. Consequently, the dynamic spin structure factor Im χ (q ,ω ) is nonzero at frequencies above the single-particle continuum. In the boson language, this effect results from the marginally irrelevant backscattering operator of the sine-Gordon model. Away from the threshold, the high-frequency tail of Im χ (q ,ω ) due to backscattering is larger than that due to finite mass by a factor of kF/q . We derive the renormalization group equations for the coupling constants of the g -ology model at finite ω and q and find the corresponding expression for χ (q ,ω ) , valid to all orders in the interaction but not in the immediate vicinity of the continuum boundary, where the finite-mass effects become dominant.

  14. Mechanical Assessment of the Drep Shield Subject to Vibratory Motion and Dynamic and Static Rock Loading

    SciTech Connect

    R.C. Quittmeyer

    2005-11-16

    The purpose of the drip shield (DS) is to divert water that may seep into emplacement drifts from contacting the waste packages, and to protect the waste packages from impact or static loading from rockfall. The objective of this document is to summarize, into one location, the results of a series of supporting engineering calculations that were developed to study the effect of static and dynamic loads on the mechanical performance of the DS. The potential DS loads are a result of: (1) Potential earthquake vibratory ground motion, and resulting interaction of the DS, waste package and pallet, and drift invert; (2) Dynamic impacts of rockfall resulting from emplacement drift damage as a result of earthquake vibratory motion; and (3) Static load of the caved rock rubble that may come to rest on the DS as a result of vibratory motion or from time-dependent yielding of the rock mass surrounding the emplacement drift. The potential mechanical failure mechanisms that may result from these loads include: (1) Overturning and/or separation of the interlocking DS segments; (2) Loss of structural integrity and stability of the DS, including excessive deformation or buckling; and (3) Localized damage to the top and side-wall plates of the DS. The scope of this document is limited to summarizing results presented in the supporting calculations in the areas of analysis of the potential for DS collapse, and determination of the damaged surface area of the DS plates. New calculations are presented to determine whether or not separation of DSs occur under vibratory motion.

  15. Non-diffusive spin dynamics in a two-dimensional electron gas

    SciTech Connect

    Weber, C.P.

    2010-04-28

    We describe measurements of spin dynamics in the two-dimensional electron gas in GaAs/GaAlAs quantum wells. Optical techniques, including transient spin-grating spectroscopy, are used to probe the relaxation rates of spin polarization waves in the wavevector range from zero to 6 x 10{sup 4} cm{sup -1}. We find that the spin polarization lifetime is maximal at nonzero wavevector, in contrast with expectation based on ordinary spin diffusion, but in quantitative agreement with recent theories that treat diffusion in the presence of spin-orbit coupling.

  16. Dynamical spin injection at a quasi-one-dimensional ferromagnet-graphene interface

    SciTech Connect

    Singh, S.; Ahmadi, A.; Mucciolo, E. R.; Barco, E. del; Cherian, C. T.; Özyilmaz, B.

    2015-01-19

    We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a signature of dynamical spin injection, wherein a pure spin current is pumped into the single-layer graphene from the precessing magnetization of the ferromagnet. The observed spin pumping efficiency is difficult to reconcile with the expected backflow of spins according to the standard spin pumping theory and the characteristics of graphene, and constitutes an enigma for spin pumping in two-dimensional structures.

  17. Influence of temperature on spin polarization dynamics in dilute nitride semiconductors—Role of nonparamagnetic centers

    SciTech Connect

    Baranowski, M.; Misiewicz, J.

    2015-10-21

    We report theoretical studies of spin polarization dynamics in dilute nitride semiconductors. We develop a commonly used rate equation model [Lagarde et al., Phys. Status Solidi A 204, 208 (2007) and Kunold et al. Phys. Rev. B 83, 165202 (2011)] to take into account the influence of shallow localizing states on the temperature dependence of spin polarization dynamics and a spin filtering effect. Presented investigations show that the experimentally observed temperature dependence of a spin polarization lifetime in dilute nitrides can be related to the electron capture process by shallow localizing states without paramagnetic properties. This process reduces the efficiency of spin filtering effect by deep paramagnetic centers, especially at low temperatures.

  18. Phonon-magnon interactions in BCC iron: A combined molecular and spin dynamics study

    SciTech Connect

    Perera, Meewanage Dilina N; Landau, David P; Nicholson, Don M; Stocks, George Malcolm; Eisenbach, Markus; Yin, Junqi; Brown, Greg

    2014-01-01

    Combining an atomistic many-body potential with a classical spin Hamiltonian pa- rameterized by first principles calculations, molecular-spin dynamics computer sim- ulations were performed to investigate phonon-magnon interactions in BCC iron. Results obtained for spin-spin and density-density dynamic structure factors show that noticeable softening and damping of magnon modes occur due to the presence of lattice vibrations. Furthermore, as a result of the phonon-magnon coupling, addi- tional longitudinal spin wave excitations are observed, with the same frequencies as the longitudinal phonon modes.

  19. Influence of temperature on spin polarization dynamics in dilute nitride semiconductors—Role of nonparamagnetic centers

    NASA Astrophysics Data System (ADS)

    Baranowski, M.; Misiewicz, J.

    2015-10-01

    We report theoretical studies of spin polarization dynamics in dilute nitride semiconductors. We develop a commonly used rate equation model [Lagarde et al., Phys. Status Solidi A 204, 208 (2007) and Kunold et al. Phys. Rev. B 83, 165202 (2011)] to take into account the influence of shallow localizing states on the temperature dependence of spin polarization dynamics and a spin filtering effect. Presented investigations show that the experimentally observed temperature dependence of a spin polarization lifetime in dilute nitrides can be related to the electron capture process by shallow localizing states without paramagnetic properties. This process reduces the efficiency of spin filtering effect by deep paramagnetic centers, especially at low temperatures.

  20. Phonon-magnon interactions in body centered cubic iron: A combined molecular and spin dynamics study

    SciTech Connect

    Perera, Dilina Landau, David P.; Nicholson, Don M.; Malcolm Stocks, G.; Eisenbach, Markus; Yin, Junqi; Brown, Gregory

    2014-05-07

    Combining an atomistic many-body potential with a classical spin Hamiltonian parameterized by first principles calculations, molecular-spin dynamics computer simulations were performed to investigate phonon-magnon interactions in body centered cubic iron. Results obtained for spin-spin and density-density dynamic structure factors show that noticeable softening and damping of magnon modes occur due to the presence of lattice vibrations. Furthermore, as a result of the phonon-magnon coupling, additional longitudinal spin wave excitations are observed, with the same frequencies as the longitudinal phonon modes.

  1. Optimization of 1H spin density for dynamic nuclear polarization using photo-excited triplet electron spins.

    PubMed

    Kagawa, Akinori; Murokawa, Yu; Takeda, Kazuyuki; Kitagawa, Masahiro

    2009-03-01

    In dynamic nuclear polarization (DNP) using photo-excited triplet electron spins, known as Microwave-Induced Optical Nuclear Polarization (MIONP), the attainable (1)H polarization is determined by the ratio of the buildup rate and the spin-lattice relaxation rate, in turn depend on the (1)H spin density. It is shown that the final (1)H polarization can be enhanced by diluting the (1)H spins with partial deuteration. The DNP experiments are demonstrated in 0.05 mol% pentacene-doped p-terphenyl for various (1)H abundances. It is also shown that the (1)H spin diffusion coefficient can be determined by examining the initial buildup rate of (1)H polarization for various repetition rates of the DNP sequence.

  2. Spin-Entry Characteristics of a Large Supersonic Bomber as Determined by Dynamic Model Tests

    NASA Technical Reports Server (NTRS)

    Bowman, James S.

    1965-01-01

    An investigation has been conducted in the Langley spin tunnel and at a catapult launch facility of a 1/60-scale dynamic model to determine the spin-entry characteristics of a large supersonic bomber. Catapult tests indicated that spin-entry motions were obtainable for a center-of-gravity location of 0.21 mean aerodynamic chord but were not obtainable at a center-of-gravity location of 0.25 mean aerodynamic chord. Deflected ailerons were effective in promoting or preventing the spin- entry motion and this effect was qualitatively the same as it was for the fully developed spin. Varying the configuration had little significant effect on the spin-entry characteristics. Brief tests conducted with the model in the Langley spin tunnel indicated that fully developed spins were obtainable at the forward center-of-gravity location and that spins were highly unlikely at the rearward center-of-location.

  3. Strain dependent electron spin dynamics in bulk cubic GaN

    SciTech Connect

    Schaefer, A.; Buß, J. H.; Hägele, D.; Rudolph, J.; Schupp, T.; Zado, A.; As, D. J.

    2015-03-07

    The electron spin dynamics under variable uniaxial strain is investigated in bulk cubic GaN by time-resolved magneto-optical Kerr-rotation spectroscopy. Spin relaxation is found to be approximately independent of the applied strain, in complete agreement with estimates for Dyakonov-Perel spin relaxation. Our findings clearly exclude strain-induced relaxation as an effective mechanism for spin relaxation in cubic GaN.

  4. Strain dependent electron spin dynamics in bulk cubic GaN

    NASA Astrophysics Data System (ADS)

    Schaefer, A.; Buß, J. H.; Schupp, T.; Zado, A.; As, D. J.; Hägele, D.; Rudolph, J.

    2015-03-01

    The electron spin dynamics under variable uniaxial strain is investigated in bulk cubic GaN by time-resolved magneto-optical Kerr-rotation spectroscopy. Spin relaxation is found to be approximately independent of the applied strain, in complete agreement with estimates for Dyakonov-Perel spin relaxation. Our findings clearly exclude strain-induced relaxation as an effective mechanism for spin relaxation in cubic GaN.

  5. Imaging Spin Dynamics in Monolayer WS2 by Time-Resolved Kerr Rotation Microscopy

    NASA Astrophysics Data System (ADS)

    Bushong, Elizabeth; Luo, Kelly (Yunqiu); McCreary, Kathleen; Newburger, Michael; Singh, Simranjeet; Jonker, Berend; Kawakami, Roland

    Monolayer transition metal dichalcogenides (TMDs) such as WS2 offer a unique platform to probe spin and valley degrees of freedom in two-dimensional condensed matter systems. TMDs are of great interest because they have a direct band gap and optical selection rules that permit the excitation of both valley and spin-polarized electrons. Strong spin-orbit coupling leads to valley-dependent spin-splitting in both the conduction and valence bands, which may suppress spin relaxation and inhibit intervalley scattering, thereby increasing both the spin and valley lifetimes. To measure spin and valley dynamics of CVD grown WS2, we developed time-resolved Kerr rotation microscopy with spatial resolution of ~1 micron and temporal resolution of 150 fs. We observe a long spin lifetime of 5.1 ns in WS2 at T = 6.5 K. We spatially map the spin populations at a given time delay, and observe a complex spatial dependence of the spin lifetimes with regions of spin lifetime less than 100 ps and regions of spin lifetime greater than 5 ns separated by only a few microns. To understand the origin of the long-lived spin states, we investigate the relationship between spin lifetime and the photoluminescence intensity. Application of in-plane magnetic fields shows an oscillatory and non-oscillatory component, indicating two spin populations that experience different effective fields.

  6. Neutron spin-echo study of the critical dynamics of spin-5/2 antiferromagnets in two and three dimensions

    NASA Astrophysics Data System (ADS)

    Tseng, K. F.; Keller, T.; Walters, A. C.; Birgeneau, R. J.; Keimer, B.

    2016-07-01

    We report a neutron spin-echo study of the critical dynamics in the S =5/2 antiferromagnets MnF2 and Rb2MnF4 with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the Néel temperature, TN. By taking advantage of the μ eV energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents z for both longitudinal and transverse fluctuations. In MnF2, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents z in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb2MnF4 , the critical dynamics crosses over from the expected 2D Heisenberg behavior for T ≫TN to a scaling regime with exponent z =1.387 (4 ) , which has not been predicted by theory and may indicate the influence of long-range dipolar interactions.

  7. High temperature electron spin dynamics in bulk cubic GaN: Nanosecond spin lifetimes far above room-temperature

    NASA Astrophysics Data System (ADS)

    Buß, J. H.; Schaefer, A.; Schupp, T.; As, D. J.; Hägele, D.; Rudolph, J.

    2014-11-01

    The electron spin dynamics in n-doped bulk cubic GaN is investigated for very high temperatures from 293 K up to 500 K by time-resolved Kerr-rotation spectroscopy. We find extraordinarily long spin lifetimes exceeding 1 ns at 500 K. The temperature dependence of the spin relaxation time is in qualitative agreement with predictions of Dyakonov-Perel theory, while the absolute experimental times are an order of magnitude shorter than predicted. Possible reasons for this discrepancy are discussed, including the role of phase mixtures of hexagonal and cubic GaN as well as the impact of localized carriers.

  8. Solid effect in magic angle spinning dynamic nuclear polarization

    NASA Astrophysics Data System (ADS)

    Corzilius, Björn; Smith, Albert A.; Griffin, Robert G.

    2012-08-01

    For over five decades, the solid effect (SE) has been heavily utilized as a mechanism for performing dynamic nuclear polarization (DNP). Nevertheless, it has not found widespread application in contemporary, high magnetic field DNP experiments because SE enhancements display an ω _0 ^{ - 2} field dependence. In particular, for nominally forbidden zero and double quantum SE transitions to be partially allowed, it is necessary for mixing of adjacent nuclear spin states to occur, and this leads to the observed field dependence. However, recently we have improved our instrumentation and report here an enhancement of ɛ = 91 obtained with the organic radical trityl (OX063) in magic angle spinning experiments performed at 5 T and 80 K. This is a factor of 6-7 higher than previous values in the literature under similar conditions. Because the solid effect depends strongly on the microwave field strength, we attribute this large enhancement to larger microwave field strengths inside the sample volume, achieved with more efficient coupling of the gyrotron to the sample chamber. In addition, we develop a theoretical model to explain the dependence of the buildup rate of enhanced nuclear polarization and the steady-state enhancement on the microwave power. Buildup times and enhancements were measured as a function of 1H concentration for both trityl and Gd-DOTA. Comparison of the results indicates that for trityl the initial polarization step is the slower, rate-determining step. However, for Gd-DOTA the spread of nuclear polarization via homonuclear 1H spin diffusion is rate-limiting. Finally, we discuss the applicability of the solid effect at fields > 5 T and the requirements to address the unfavorable field dependence of the solid effect.

  9. Manipulating magnetic anisotropy and ultrafast spin dynamics of magnetic nanostructures

    NASA Astrophysics Data System (ADS)

    Cheng, Zhao-Hua; He, Wei; Zhang, Xiang-Qun; Sun, Da-Li; Du, Hai-Feng; Wu, Qiong; Ye, Jun; Fang, Ya-Peng; Liu, Hao-Liang

    2015-07-01

    We present our extensive research into magnetic anisotropy. We tuned the terrace width of Si(111) substrate by a novel method: varying the direction of heating current and consequently manipulating the magnetic anisotropy of magnetic structures on the stepped substrate by decorating its atomic steps. Laser-induced ultrafast demagnetization of a CoFeB/MgO/CoFeB magnetic tunneling junction was explored by the time-resolved magneto-optical Kerr effect (TR-MOKE) for both the parallel state (P state) and the antiparallel state (AP state) of the magnetizations between two magnetic layers. It was observed that the demagnetization time is shorter and the magnitude of demagnetization is larger in the AP state than those in the P state. These behaviors are attributed to the ultrafast spin transfer between two CoFeB layers via the tunneling of hot electrons through the MgO barrier. Our observation indicates that ultrafast demagnetization can be engineered by the hot electron tunneling current. This opens the door to manipulate the ultrafast spin current in magnetic tunneling junctions. Furthermore, an all-optical TR-MOKE technique provides the flexibility for exploring the nonlinear magnetization dynamics in ferromagnetic materials, especially with metallic materials. Project supported by the National Basic Research Program of China (Grant Nos. 2015CB921403, 2011CB921801, and 2012CB933101) and the National Natural Science Foundation of China (Grant Nos. 51427801, 11374350, 51201179, and 11274361).

  10. Imaging intracellular protein dynamics by spinning disk confocal microscopy

    PubMed Central

    Stehbens, Samantha; Pemble, Hayley; Murrow, Lindsay; Wittmann, Torsten

    2012-01-01

    The palette of fluorescent proteins has grown exponentially over the last decade, and as a result live imaging of cells expressing fluorescently tagged proteins is becoming more and more main stream. Spinning disk confocal microscopy (SDC) is a high speed optical sectioning technique, and a method of choice to observe and analyze intracellular fluorescent protein dynamics at high spatial and temporal resolution. In an SDC system, a rapidly rotating pinhole disk generates thousands of points of light that scan the specimen simultaneously, which allows direct capture of the confocal image with low noise scientific grade cooled charged-coupled device (CCD) cameras, and can achieve frame rates of up 1000 frames per second. In this chapter we describe important components of a state-of-the-art spinning disk system optimized for live cell microscopy, and provide a rationale for specific design choices. We also give guidelines how other imaging techniques such as total internal reflection (TIRF) microscopy or spatially controlled photoactivation can be coupled with SDC imaging, and provide a short protocol on how to generate cell lines stably expressing fluorescently tagged proteins by lentivirus-mediated transduction. PMID:22264541

  11. Real time dynamic behavior of vertex frustrated artificial spin ice

    NASA Astrophysics Data System (ADS)

    Lao, Yuyang; Sklenar, Joseph; Gilbert, Ian; Carrasquilo, Isaac; Scholl, Andreas; Young, Anthony; Nisoli, Cristiano; Schiffer, Peter

    Artificial spin ice systems comprise two dimensional arrays of nanoscale single domain ferromagnets designed to have frustrated interactions among the moments. By decimating islands from the common square artificial spin ice, one can design lattices with so called `vertex frustration'. In such lattices, the geometry prevents all vertices from occupying local ground states simultaneously. Using Photoemission Electron Microscopy (PEEM), we access the real time thermally induced dynamics of the moment behavior in those lattices. Operating at a proper temperature, the moment direction of each island fluctuates with a sufficiently slow frequency that it can be resolvable by acquiring successive PEEM images. We can extract information regarding the collective excitations of the moments and understand how they reflect the frustration of lattice. Supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division under Grant No. DE-SC0010778. The work of C.N. was carried out under the auspices of the US Department of Energy at LANL under Contract no. DE-AC52-06NA253962. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract no. DE-AC02-05CH11231.

  12. Spin dynamics in relativistic light-matter interaction

    NASA Astrophysics Data System (ADS)

    Bauke, Heiko; Ahrens, Sven; Keitel, Christoph H.; Grobe, Rainer

    2015-05-01

    Various spin effects are expected to become observable in light-matter interaction at relativistic intensities. Relativistic quantum mechanics equipped with a suitable relativistic spin operator forms the theoretical foundation for describing these effects. Various proposals for relativistic spin operators have been offered by different authors, which are presented in a unified way. As a result of the operators' mathematical properties only the Foldy-Wouthuysen operator and the Pryce operator qualify as possible proper relativistic spin operators. The ground states of highly charged hydrogen-like ions can be utilized to identify a legitimate relativistic spin operator experimentally. Subsequently, the Foldy-Wouthuysen spin operator is employed to study electron-spin precession in high-intensity standing light waves with elliptical polarization. For a correct theoretical description of the predicted electron-spin precession relativistic effects due to the spin angular momentum of the electromagnetic wave has to be taken into account even in the limit of low intensities.

  13. Dynamics of Spin-Orbit Coupled Bose-Einstein Condensates in a Random Potential.

    PubMed

    Mardonov, Sh; Modugno, M; Sherman, E Ya

    2015-10-30

    Disorder plays a crucial role in spin dynamics in solids and condensed matter systems. We demonstrate that for a spin-orbit coupled Bose-Einstein condensate in a random potential two mechanisms of spin evolution that can be characterized as "precessional" and "anomalous" are at work simultaneously. The precessional mechanism, typical for solids, is due to the condensate displacement. The unconventional anomalous mechanism is due to the spin-dependent velocity producing the distribution of the condensate spin polarization. The condensate expansion is accompanied by a random displacement and fragmentation, where it becomes sparse, as clearly revealed in the spin dynamics. Thus, different stages of the evolution can be characterized by looking at the condensate spin.

  14. Dynamics of Spin-Orbit Coupled Bose-Einstein Condensates in a Random Potential

    NASA Astrophysics Data System (ADS)

    Mardonov, Sh.; Modugno, M.; Sherman, E. Ya.

    2015-10-01

    Disorder plays a crucial role in spin dynamics in solids and condensed matter systems. We demonstrate that for a spin-orbit coupled Bose-Einstein condensate in a random potential two mechanisms of spin evolution that can be characterized as "precessional" and "anomalous" are at work simultaneously. The precessional mechanism, typical for solids, is due to the condensate displacement. The unconventional anomalous mechanism is due to the spin-dependent velocity producing the distribution of the condensate spin polarization. The condensate expansion is accompanied by a random displacement and fragmentation, where it becomes sparse, as clearly revealed in the spin dynamics. Thus, different stages of the evolution can be characterized by looking at the condensate spin.

  15. Spin dynamics of an individual Cr atom in a semiconductor quantum dot under optical excitation

    NASA Astrophysics Data System (ADS)

    Lafuente-Sampietro, A.; Utsumi, H.; Boukari, H.; Kuroda, S.; Besombes, L.

    2016-08-01

    We studied the spin dynamics of a Cr atom incorporated in a II-VI semiconductor quantum dot using photon correlation techniques. We used recently developed singly Cr-doped CdTe/ZnTe quantum dots to access the spin of an individual magnetic atom. Auto-correlation of the photons emitted by the quantum dot under continuous wave optical excitation reveals fluctuations of the localized spin with a timescale in the 10 ns range. Cross-correlation gives quantitative transfer time between Cr spin states. A calculation of the time dependence of the spin levels population in Cr-doped quantum dots shows that the observed spin dynamics is dominated by the exciton-Cr interaction. These measurements also provide a lower bound in the 20 ns range for the intrinsic Cr spin relaxation time.

  16. Generation of spin-polarized currents via cross-relaxation with dynamically pumped paramagnetic impurities

    SciTech Connect

    Meriles, Carlos A.; Doherty, Marcus W.

    2014-07-14

    Key to future spintronics and spin-based information processing technologies is the generation, manipulation, and detection of spin polarization in a solid state platform. Here, we theoretically explore an alternative route to spin injection via the use of dynamically polarized nitrogen-vacancy (NV) centers in diamond. We focus on the geometry where carriers and NV centers are confined to proximate, parallel layers and use a “trap-and-release” model to calculate the spin cross-relaxation probabilities between the charge carriers and neighboring NV centers. We identify near-unity regimes of carrier polarization depending on the NV spin state, applied magnetic field, and carrier g-factor. In particular, we find that unlike holes, electron spins are distinctively robust against spin-lattice relaxation by other, unpolarized paramagnetic centers. Further, the polarization process is only weakly dependent on the carrier hopping dynamics, which makes this approach potentially applicable over a broad range of temperatures.

  17. Dynamics of two coupled semiconductor spin qubits in a noisy environment

    NASA Astrophysics Data System (ADS)

    Das Sarma, S.; Throckmorton, Robert E.; Wu, Yang-Le

    2016-07-01

    We theoretically consider the temporal dynamics of two coupled spin qubits (e.g., semiconductor quantum dots) driven by the interqubit spin-spin coupling. The presence of environmental noise (e.g., charge traps, nuclear spins, random magnetic impurities) is accounted for by including random magnetic field and random interqubit coupling terms in the Hamiltonian. Both Heisenberg coupling and Ising coupling between the spin qubits are considered, corresponding respectively to exchange and capacitive gates as appropriate for single spin and singlet-triplet semiconductor qubit systems, respectively. Both exchange (Heisenberg) and capacitive (Ising) coupling situations can be solved numerically exactly even in the presence of noise, leading to the key findings that (i) the steady-state return probability to the initial state remains close to unity in the presence of strong noise for many, but not all, starting spin configurations, and (ii) the return probability as a function of time is oscillatory with a characteristic noise-controlled decay toward the steady-state value. We also provide results for the magnetization dynamics of the coupled two-qubit system. Our predicted dynamics can be directly tested in the already existing semiconductor spin qubit setups providing insight into their coherent interaction dynamics. Retention of the initial state spin memory even in the presence of strong environmental noise has important implications for quantum computation using spin qubits.

  18. Electrical manipulation of dynamic magnetic impurity and spin texture of helical Dirac fermions

    NASA Astrophysics Data System (ADS)

    Wang, Rui-Qiang; Zhong, Min; Zheng, Shi-Han; Yang, Mou; Wang, Guang-Hui

    2016-05-01

    We have theoretically investigated the spin inelastic scattering of helical electrons off a high-spin nanomagnet absorbed on a topological surface. The nanomagnet is treated as a dynamic quantum spin and driven by the spin transfer torque effect. We proposed a mechanism to electrically manipulate the spin texture of helical Dirac fermions rather than by an external magnetic field. By tuning the bias voltage and the direction of impurity magnetization, we present rich patterns of spin texture, from which important fingerprints exclusively associated with the spin helical feature are obtained. Furthermore, it is found that the nonmagnetic potential can create the resonance state in the spin density with different physics as the previously reported resonance of charge density.

  19. Dynamical theory of spin noise and relaxation: Prospects for real-time NMR measurements.

    PubMed

    Field, Timothy R

    2014-11-01

    Recent developments in theoretical aspects of spin noise and relaxation and their interrelationship reveal a modified spin density, distinct from the density matrix, as the necessary object to describe fluctuations in spin systems. These fluctuations are to be viewed as an intrinsic quantum mechanical property of such systems immersed in random magnetic environments and are observed as "spin noise" in the absence of any radio frequency excitation. With the prospect of ultrafast digitization, the role of spin noise in real-time parameter extraction for (NMR) spin systems, and the advantage over standard techniques, is of essential importance, especially for systems containing a small number of spins. In this article we outline prospects for harnessing the recent dynamical theory in terms of spin-noise measurement, with attention to real-time properties.

  20. Optically controlled electron-nuclear spin dynamics in a quantum dot

    NASA Astrophysics Data System (ADS)

    Barnes, Edwin; Economou, Sophia

    2011-03-01

    In recent years, a large number of experiments involving coherent and incoherent control of electron spins in quantum dots have revealed the important role of the nuclear spins of the host material. Experiments with optical controls, both pulsed and continuous wave, have shown that the feedback of the nuclear spins on the electron spin strongly affects the electron spin response. However, a microscopic theory of this mechanism is not available at present. We introduce a formalism that allows us to investigate this system without invoking any phenomenological spin-flip rates for the nuclei. We derive the electron-nuclear dynamics under the influence of external periodic pulsed control to second order in the electron-nuclear hyperfine coupling. Our formalism should have wide applications in both coherently and incoherently driven electron spins interacting with a nuclear spin bath, including self-assembled and gated quantum dots. Work (EB) supported by LPS-CMTC and CNAM.

  1. Quench dynamics and statistics of measurements for a line of quantum spins in two dimensions

    NASA Astrophysics Data System (ADS)

    Lux, Jonathan; Rosch, Achim

    2015-02-01

    Motivated by recent experiments, we investigate the dynamics of a line of spin-down spins embedded in the ferromagnetic spin-up ground state of a two-dimensional XXZ model close to the Ising limit. In a situation where the couplings in the x and y directions are different, the quench dynamics of this system is governed by the interplay of one-dimensional excitations (kinks and holes) moving along the line and single-spin excitations evaporating into the two-dimensional background. A semiclassical approximation can be used to calculate the dynamics of this complex quantum system. Recently, it became possible to perform projective quantum measurements on such spin systems, allowing us to determine, e.g., the z component of each individual spin. We predict the statistical properties of such measurements which contain much more information than correlation functions.

  2. Measurement backaction on the quantum spin-mixing dynamics of a spin-1 Bose-Einstein condensate

    SciTech Connect

    Zhang Keye; Zhou Lu; Zhang Weiping; Ling, Hong Y.; Pu Han

    2011-06-15

    We consider a small F=1 spinor condensate inside an optical cavity driven by an optical probe field, and subject the output of the probe to a homodyne detection, with the goal of investigating the effect of measurement backaction on the spin dynamics of the condensate. Using the stochastic master equation approach, we show that the effect of backaction is sensitive to not only the measurement strength but also the quantum fluctuation of the spinor condensate. The same method is also used to estimate the atom numbers below which the effect of backaction becomes so prominent that extracting spin dynamics from this cavity-based detection scheme is no longer practical.

  3. Spin component-scaled second-order Møller-Plesset perturbation theory for calculating NMR shieldings.

    PubMed

    Maurer, Marina; Ochsenfeld, Christian

    2015-01-13

    Spin component-scaled and scaled opposite-spin second-order Møller-Plesset perturbation approaches (SCS-MP2 and SOS-MP2) are introduced for calculating NMR chemical shifts in analogy to the well-established scaled approaches for MP2 energies. Gauge-including atomic orbitals (GIAO) are employed throughout this work. The GIAO-SCS-MP2 and GIAO-SOS-MP2 methods typically show superior performance to nonscaled MP2 and are closer to the coupled-cluster singles doubles perturbative triples (CCSD(T))/cc-pVQZ reference values. In addition, the pragmatic use of mixed basis sets for the Hartree-Fock and the correlated part of NMR chemical shift calculations is shown to be beneficial. PMID:26574201

  4. Dynamics of domain wall driven by spin-transfer torque

    SciTech Connect

    Chureemart, P.; Evans, R. F. L.; Chantrell, R. W.

    2011-05-01

    Spin-torque switching of magnetic devices offers new technological possibilities for data storage and integrated circuits. We have investigated domain-wall motion in a ferromagnetic thin film driven by a spin-polarized current using an atomistic spin model with a modified Landau-Lifshitz-Gilbert equation including the effect of the spin-transfer torque. The presence of the spin-transfer torque is shown to create an out-of-plane domain wall, in contrast to the external-field-driven case where an in-plane wall is found. We have investigated the effect of the spin torque on domain-wall displacement, domain-wall velocity, and domain-wall width, as well as the equilibration time in the presence of the spin-transfer torque. We have shown that the minimum spin-current density, regarded as the critical value for domain-wall motion, decreases with increasing temperature.

  5. Theoretical gas to liquid shift of (15)N isotropic nuclear magnetic shielding in nitromethane using ab initio molecular dynamics and GIAO/GIPAW calculations.

    PubMed

    Gerber, Iann C; Jolibois, Franck

    2015-05-14

    Chemical shift requires the knowledge of both the sample and a reference magnetic shielding. In few cases as nitrogen (15N), the standard experimental reference corresponds to its liquid phase. Theoretical estimate of NMR magnetic shielding parameters of compounds in their liquid phase is then mandatory but usually replaced by an easily-get gas phase value, forbidding direct comparisons with experiments. We propose here to combine ab initio molecular dynamic simulations with the calculations of magnetic shielding using GIAO approach on extracted cluster's structures from MD. Using several computational strategies, we manage to accurately calculate 15N magnetic shielding of nitromethane in its liquid phase. Theoretical comparison between liquid and gas phase allows us to extrapolate an experimental value for the 15N magnetic shielding of nitromethane in gas phase between -121.8 and -120.8 ppm.

  6. Influence of Impurity Spin Dynamics on Quantum Transport in Epitaxial Graphene

    NASA Astrophysics Data System (ADS)

    Lara-Avila, Samuel; Kubatkin, Sergey; Kashuba, Oleksiy; Folk, Joshua A.; Lüscher, Silvia; Yakimova, Rositza; Janssen, T. J. B. M.; Tzalenchuk, Alexander; Fal'ko, Vladimir

    2015-09-01

    Experimental evidence from both spin-valve and quantum transport measurements points towards unexpectedly fast spin relaxation in graphene. We report magnetotransport studies of epitaxial graphene on SiC in a vector magnetic field showing that spin relaxation, detected using weak-localization analysis, is suppressed by an in-plane magnetic field B∥, and thereby proving that it is caused at least in part by spinful scatterers. A nonmonotonic dependence of the effective decoherence rate on B∥ reveals the intricate role of the scatterers' spin dynamics in forming the interference correction to the conductivity, an effect that has gone unnoticed in earlier weak localization studies.

  7. Self-Polarization and Dynamical Cooling of Nuclear Spins in Double Quantum Dots

    NASA Astrophysics Data System (ADS)

    Rudner, M. S.; Levitov, L. S.

    2007-07-01

    The spin-blockade regime of double quantum dots features coupled dynamics of electron and nuclear spins resulting from the hyperfine interaction. We explain observed nuclear self-polarization via a mechanism based on feedback of the Overhauser shift on electron energy levels, and propose to use the instability toward self-polarization as a vehicle for controlling the nuclear spin distribution. In the dynamics induced by a properly chosen time-dependent magnetic field, nuclear spin fluctuations can be suppressed significantly below the thermal level.

  8. Spinor dynamics in an antiferromagnetic spin-1 condensate.

    PubMed

    Black, A T; Gomez, E; Turner, L D; Jung, S; Lett, P D

    2007-08-17

    We observe coherent spin oscillations in an antiferromagnetic spin-1 Bose-Einstein condensate of sodium. The variation of the spin oscillations with magnetic field shows a clear signature of nonlinearity, in agreement with theory, which also predicts anharmonic oscillations near a critical magnetic field. Measurements of the magnetic phase diagram agree with predictions made in the approximation of a single spatial mode. The oscillation period yields the best measurement to date of the sodium spin-dependent interaction coefficient, determining that the difference between the sodium spin-dependent s-wave scattering lengths a(f=2) - a(f=0) is 2.47+/-0.27 Bohr radii.

  9. Spinor Dynamics in an Antiferromagnetic Spin-1 Condensate

    SciTech Connect

    Black, A. T.; Gomez, E.; Turner, L. D.; Jung, S.; Lett, P. D.

    2007-08-17

    We observe coherent spin oscillations in an antiferromagnetic spin-1 Bose-Einstein condensate of sodium. The variation of the spin oscillations with magnetic field shows a clear signature of nonlinearity, in agreement with theory, which also predicts anharmonic oscillations near a critical magnetic field. Measurements of the magnetic phase diagram agree with predictions made in the approximation of a single spatial mode. The oscillation period yields the best measurement to date of the sodium spin-dependent interaction coefficient, determining that the difference between the sodium spin-dependent s-wave scattering lengths a{sub f=2}-a{sub f=0} is 2.47{+-}0.27 Bohr radii.

  10. Dynamical decoupling design for identifying weakly coupled nuclear spins in a bath

    NASA Astrophysics Data System (ADS)

    Zhao, Nan; Wrachtrup, Jörg; Liu, Ren-Bao

    2014-09-01

    Identifying weakly coupled nuclear spins around single electron spins is a key step toward implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single-spin nuclear magnetic resonance detection using diamond defect spins. Dynamical decoupling control of the center electron spin with periodic pulse sequences [e.g., the Carre-Purcell-Meiboom-Gill (CPMG) sequence] has been successfully used to identify single nuclear spins and to resolve structure of nuclear spin clusters. Here, we design a type of pulse sequence by replacing the repetition unit (a single π pulse) of the CPMG sequence with a group of nonuniformly spaced π pulses. Using the nitrogen-vacancy center system in diamond, we theoretically demonstrate that the designed pulse sequence improves the resolution of nuclear spin noise spectroscopy, and more information about the surrounding nuclear spins is extracted. The principle of dynamical decoupling design proposed in this paper is useful in many systems (e.g., defect spin qubit in solids, trapped ion, and superconducting qubit) for high-resolution noise spectroscopy.

  11. Spinach - A software library for simulation of spin dynamics in large spin systems

    NASA Astrophysics Data System (ADS)

    Hogben, H. J.; Krzystyniak, M.; Charnock, G. T. P.; Hore, P. J.; Kuprov, Ilya

    2011-02-01

    We introduce a software library incorporating our recent research into efficient simulation algorithms for large spin systems. Liouville space simulations (including symmetry, relaxation and chemical kinetics) of most liquid-state NMR experiments on 40+ spin systems can now be performed without effort on a desktop workstation. Much progress has also been made with improving the efficiency of ESR, solid state NMR and Spin Chemistry simulations. Spinach is available for download at http://spindynamics.org.

  12. Dynamics of the collective modes of an inhomogeneous spin ensemble in a cavity

    SciTech Connect

    Wesenberg, Janus H.; Kurucz, Zoltan; Moelmer, Klaus

    2011-02-15

    We study the excitation dynamics of an inhomogeneously broadened spin ensemble coupled to a single cavity mode. The collective excitations of the spin ensemble can be described in terms of generalized spin waves, and, in the absence of the cavity, the free evolution of the spin ensemble can be described as a drift in the wavenumber without dispersion. In this article we show that the dynamics in the presence of coupling to the cavity mode can be described solely by a modified time evolution of the wavenumbers. In particular, we show that collective excitations with a well-defined wavenumber pass without dispersion from negative to positive-valued wavenumbers without populating the zero wavenumber spin wave mode. The results are relevant for multimode collective quantum memories where qubits are encoded in different spin waves.

  13. Self-consistent description of spin-phonon dynamics in ferromagnets

    NASA Astrophysics Data System (ADS)

    Nieves, P.; Serantes, D.; Chubykalo-Fesenko, O.

    2016-07-01

    Several recently reported exciting phenomena such as spin caloritronics or ultrafast laser-induced spin dynamics involve the action of temperature on spin dynamics. However, the inverse effect of magnetization dynamics on temperature change is very frequently ignored. Based on the density matrix approach, in this work we derive a self-consistent model for describing the magnetization and phonon temperature dynamics in ferromagnets in the framework of the quantum Landau-Lifshitz-Bloch equation. We explore potential applicability of our approach for two cases, inspired by magnetocaloric effect and magnetic fluid hyperthermia. In the first case, the spin-phonon dynamics is governed by the longitudinal relaxation in bulk systems close to the Curie temperature; while in the second case it is described by the transverse relaxation during the hysteresis cycle of individual nanoparticles well below the Curie temperature.

  14. Next-to-leading order gravitational spin(1)-spin(2) dynamics in Hamiltonian form

    SciTech Connect

    Steinhoff, Jan; Hergt, Steven; Schaefer, Gerhard

    2008-04-15

    Based on recent developments by the authors a next-to-leading order spin(1)-spin(2) Hamiltonian is derived for the first time. The result is obtained within the canonical formalism of Arnowitt, Deser, and Misner (ADM) utilizing their generalized isotropic coordinates. A comparison with other methods is given.

  15. Collective dynamics of solid-state spin chains and ensembles in quantum information processing

    NASA Astrophysics Data System (ADS)

    Ping, Yuting

    This thesis is concerned with the collective dynamics in different spin chains and spin ensembles in solid-state materials. The focus is on the manipulation of electron spins, through spin-spin and spin-photon couplings controlled by voltage potentials or electromagnetic fields. A brief review of various systems is provided to describe the possible physical implementation of the ideas, and also outlines the basis of the adopted effective interaction models. The first two ideas presented explore the collective behaviour of non-interacting spin chains with external couplings. One focuses on mapping the identical state of spin-singlet pairs in two currents onto two distant, static spins downstream, creating distributed entanglement that may be accessed. The other studies a quantum memory consisting of an array of non-interacting, static spins, which may encode and decode multiple flying spins. Both chains could effectively `enhance' weak couplings in a cumulative fashion, and neither scheme requires active quantum control. Moreover, the distributed entanglement generated can offer larger separation between the qubits than more conventional protocols that only exploit the tunnelling effects between quantum dots. The quantum memory can also `smooth' the statistical fluctuations in the effects of local errors when the stored information is spread. Next, an interacting chain of static spins with nearest-neighbour interactions is introduced to connect distant end spins. Previously, it has been shown that this approach provides a cubic speed-up when compared with the direct coupling between the target spins. The practicality of this scheme is investigated by analysing realistic error effects via numerical simulations, and from that perspective relaxation of the nearest-neighbour assumption is proposed. Finally, a non-interacting electron spin ensemble is reviewed as a quantum memory to store single photons from an on-chip stripline cavity. It is then promoted to a full

  16. Dynamics of caged microemulsion droplets: a neutron spin echo and dynamic light scattering study

    NASA Astrophysics Data System (ADS)

    Geyer, Arnaud de; Molle, Boris; Lartigue, Colette; Guillermo, Armel; Farago, Bela

    2004-07-01

    We report a neutron spin echo (NSE) and dynamic light scattering (DLS) study of droplet dynamics in a microemulsion at high droplet packing fraction ( Φdroplet∼62%). NSE measurements in range qr≫1 allow to investigate the short-range Brownian motion of droplets trapped within the cages formed by their nearest neighbors. For a particular scattering contrast, NSE also reveals, for q values around qr∼ π, the shape fluctuations of the caged droplets. In range qr≪1, DLS correlation functions reveal two independent diffusive modes with well separated decay times. Comparing DLS results with NSE and pulsed-field gradient NMR measurements allows to associate both DLS modes with collective dynamics of ‘transient-trapped’ droplets, revealing strong similarity to the long-time and short-time diffusion modes observed by light scattering in concentrated colloidal suspensions below the glass transition.

  17. Spectroscopy of spontaneous spin noise as a probe of spin dynamics and magnetic resonance.

    PubMed

    Crooker, S A; Rickel, D G; Balatsky, A V; Smith, D L

    2004-09-01

    Not all noise in experimental measurements is unwelcome. Certain fundamental noise sources contain valuable information about the system itself-a notable example being the inherent voltage fluctuations (Johnson noise) that exist across any resistor, which allow the temperature to be determined. In magnetic systems, fundamental noise can exist in the form of random spin fluctuations. For example, statistical fluctuations of N paramagnetic spins should generate measurable noise of order N spins, even in zero magnetic field. Here we exploit this effect to perform perturbation-free magnetic resonance. We use off-resonant Faraday rotation to passively detect the magnetization noise in an equilibrium ensemble of paramagnetic alkali atoms; the random fluctuations generate spontaneous spin coherences that precess and decay with the same characteristic energy and timescales as the macroscopic magnetization of an intentionally polarized or driven ensemble. Correlation spectra of the measured spin noise reveal g-factors, nuclear spin, isotope abundance ratios, hyperfine splittings, nuclear moments and spin coherence lifetimes-without having to excite, optically pump or otherwise drive the system away from thermal equilibrium. These noise signatures scale inversely with interaction volume, suggesting a possible route towards non-perturbative, sourceless magnetic resonance of small systems. PMID:15343328

  18. Spin transport and dynamics in the F/N junction

    NASA Astrophysics Data System (ADS)

    Li, Hua; Bedell, Kevin

    2015-03-01

    We study the spin transport in the low temperature regime (often referred to as the precession-dominated regime) between a ferromagnetic Fermi liquid (FFL) and a normal metal metallic Fermi liquid (NFL), the F/N junction, which is considered one of the basic spintronic devices. In particular, we explore the propagation of spin waves and transport of magnetization through the interface of the F/N junction where non-equilibrium spin polarization is created on the normal metal side of the junction by spin injection. We calculate the probable spin wave modes in the precession-dominated regime on both sides of the junction especially on the NFL side where the system is out of equilibrium. Proper boundary conditions at the interface are introduced to establish the transport of the spin properties through the F/N junction. In the end, a possible transmission conduction electron spin resonance experiment is suggested on the F/N junction to see if the predicted spin wave modes could propagate through the junction.

  19. Dynamic neutron scattering on incoherent systems using efficient resonance spin flip techniques

    SciTech Connect

    Häussler, Wolfgang; Kredler, Lukas

    2014-05-15

    We have performed numerical ray-tracing Monte-Carlo-simulations of incoherent dynamic neutron scattering experiments. We intend to optimize the efficiency of incoherent measurements depending on the fraction of neutrons scattered without and with spin flip at the sample. In addition to conventional spin echo, we have numerically and experimentally studied oscillating intensity techniques. The results point out the advantages of these different spin echo variants and are an important prerequisite for neutron resonance spin echo instruments like RESEDA (FRM II, Munich), to choose the most efficient technique depending on the scattering vector range and the properties of the sample system under study.

  20. Spin dynamics of polarons and polaron pairs in a random hyperfine field

    NASA Astrophysics Data System (ADS)

    Roundy, Robert C.

    Spin-dependent recombination of polaron pairs and spin relaxation of a single polaron are the most fundamental processes are responsible for the performance of organic spintronics-based devices such as light-emitting diodes and organic spin valves. In organic materials, with no spin-orbit coupling, both processes are due to random hyperfine fields created by protons neighboring the polaron sites. The essence of spin-dependent recombination is that in order to recombine the pair must be in the singlet state. Hyperfine fields acting on the electron and hole govern the spin-dynamics of localized pairs during the waiting time for recombination. We demonstrate that for certain domain of trapping configurations of hyperfine fields, crossover to the singlet state is quenched. This leads to the blocking of current. The phenomenon of organic magnetoresistance (OMAR) is described by counting the weights of trapping configurations as a function of magnetic field. This explains the universality of the lineshapes of the OMAR curves. In finite samples incomplete averaging over the hyperfine fields gives rise to mesoscopic fluctuations of the current response. We also demonstrate that under the condition of magnetic resonance, new trapping configurations emerge. This leads to nontrivial evolution of current through the sample with microwave power. When discussing spin-relaxation two questions can be asked: (a) How does the local spin polarization decay as a function of distance from the spin-polarized injector? (b) How does the injected spin decay as a function of time after spatial averaging? With regard to (a), we demonstrate that, while decaying exponentially on average, local spin-polarization exhibits giant fluctuations from point to point. Concerning (b), we find that for a spin-carrier which moves diffusively in low dimensions the decay is faster than a simple exponent. The underlying physics for both findings is that in describing spin evolution it is necessary to add up

  1. Lattice Dynamics of EuO: Evidence for Giant Spin-Phonon Coupling

    NASA Astrophysics Data System (ADS)

    Pradip, R.; Piekarz, P.; Bosak, A.; Merkel, D. G.; Waller, O.; Seiler, A.; Chumakov, A. I.; Rüffer, R.; Oleś, A. M.; Parlinski, K.; Krisch, M.; Baumbach, T.; Stankov, S.

    2016-05-01

    Comprehensive studies of lattice dynamics in the ferromagnetic semiconductor EuO have been performed by a combination of inelastic x-ray scattering, nuclear inelastic scattering, and ab initio calculations. A remarkably large broadening of the transverse acoustic phonons was discovered at temperatures above and below the Curie temperature TC=69 K . This result indicates a surprisingly strong momentum-dependent spin-phonon coupling induced by the spin dynamics in EuO.

  2. High temperature spin dynamics in linear magnetic chains, molecular rings, and segments by nuclear magnetic resonance

    NASA Astrophysics Data System (ADS)

    Adelnia, Fatemeh; Mariani, Manuel; Ammannato, Luca; Caneschi, Andrea; Rovai, Donella; Winpenny, Richard; Timco, Grigore; Corti, Maurizio; Lascialfari, Alessandro; Borsa, Ferdinando

    2015-05-01

    We present the room temperature proton nuclear magnetic resonance (NMR) nuclear spin-lattice relaxation rate (NSLR) results in two 1D spin chains: the Heisenberg antiferromagnetic (AFM) Eu(hfac)3NITEt and the magnetically frustrated Gd(hfac)3NITEt. The NSLR as a function of external magnetic field can be interpreted very well in terms of high temperature spin dynamics dominated by a long time persistence of the decay of the two-spin correlation function due to the conservation of the total spin value for isotropic Heisenberg chains. The high temperature spin dynamics are also investigated in Heisenberg AFM molecular rings. In both Cr8 closed ring and in Cr7Cd and Cr8Zn open rings, i.e., model systems for a finite spin segment, an enhancement of the low frequency spectral density is found consistent with spin diffusion but the high cut-off frequency due to intermolecular anisotropic interactions prevents a detailed analysis of the spin diffusion regime.

  3. High temperature spin dynamics in linear magnetic chains, molecular rings, and segments by nuclear magnetic resonance

    SciTech Connect

    Adelnia, Fatemeh; Lascialfari, Alessandro; Mariani, Manuel; Ammannato, Luca; Caneschi, Andrea; Rovai, Donella; Winpenny, Richard; Timco, Grigore; Corti, Maurizio Borsa, Ferdinando

    2015-05-07

    We present the room temperature proton nuclear magnetic resonance (NMR) nuclear spin-lattice relaxation rate (NSLR) results in two 1D spin chains: the Heisenberg antiferromagnetic (AFM) Eu(hfac){sub 3}NITEt and the magnetically frustrated Gd(hfac){sub 3}NITEt. The NSLR as a function of external magnetic field can be interpreted very well in terms of high temperature spin dynamics dominated by a long time persistence of the decay of the two-spin correlation function due to the conservation of the total spin value for isotropic Heisenberg chains. The high temperature spin dynamics are also investigated in Heisenberg AFM molecular rings. In both Cr{sub 8} closed ring and in Cr{sub 7}Cd and Cr{sub 8}Zn open rings, i.e., model systems for a finite spin segment, an enhancement of the low frequency spectral density is found consistent with spin diffusion but the high cut-off frequency due to intermolecular anisotropic interactions prevents a detailed analysis of the spin diffusion regime.

  4. Spin dynamics and relaxation in graphene dictated by electron-hole puddles

    PubMed Central

    Van Tuan, Dinh; Ortmann, Frank; Cummings, Aron W.; Soriano, David; Roche, Stephan

    2016-01-01

    The understanding of spin dynamics and relaxation mechanisms in clean graphene, and the upper time and length scales on which spin devices can operate, are prerequisites to realizing graphene-based spintronic technologies. Here we theoretically reveal the nature of fundamental spin relaxation mechanisms in clean graphene on different substrates with Rashba spin-orbit fields as low as a few tens of μeV. Spin lifetimes ranging from 50 picoseconds up to several nanoseconds are found to be dictated by substrate-induced electron-hole characteristics. A crossover in the spin relaxation mechanism from a Dyakonov-Perel type for SiO2 substrates to a broadening-induced dephasing for hBN substrates is described. The energy dependence of spin lifetimes, their ratio for spins pointing out-of-plane and in-plane, and the scaling with disorder provide a global picture about spin dynamics and relaxation in ultraclean graphene in the presence of electron-hole puddles. PMID:26876333

  5. Spin dynamics and relaxation in graphene dictated by electron-hole puddles.

    PubMed

    Tuan, Dinh Van; Ortmann, Frank; Cummings, Aron W; Soriano, David; Roche, Stephan

    2016-01-01

    The understanding of spin dynamics and relaxation mechanisms in clean graphene, and the upper time and length scales on which spin devices can operate, are prerequisites to realizing graphene-based spintronic technologies. Here we theoretically reveal the nature of fundamental spin relaxation mechanisms in clean graphene on different substrates with Rashba spin-orbit fields as low as a few tens of μeV. Spin lifetimes ranging from 50 picoseconds up to several nanoseconds are found to be dictated by substrate-induced electron-hole characteristics. A crossover in the spin relaxation mechanism from a Dyakonov-Perel type for SiO2 substrates to a broadening-induced dephasing for hBN substrates is described. The energy dependence of spin lifetimes, their ratio for spins pointing out-of-plane and in-plane, and the scaling with disorder provide a global picture about spin dynamics and relaxation in ultraclean graphene in the presence of electron-hole puddles. PMID:26876333

  6. Probing dynamics of a spin ensemble of P1 centers in diamond using a superconducting resonator

    NASA Astrophysics Data System (ADS)

    de Lange, Gijs; Ranjan, Vishal; Schutjens, Ron; Debelhoir, Thibault; Groen, Joost; Szombati, Daniel; Thoen, David; Klapwijk, Teun; Hanson, Ronald; Dicarlo, Leonardo

    2013-03-01

    Solid-state spin ensembles are promising candidates for realizing a quantum memory for superconducting circuits. Understanding the dynamics of such ensembles is a necessary step towards achieving this goal. Here, we investigate the dynamics of an ensemble of nitrogen impurities (P1 centers) in diamond using magnetic-field controlled coupling to the first two modes of a superconducting (NbTiN) coplanar waveguide resonator. Three hyperfine-split spin sub-ensembles are clearly resolved in the 0.25-1.2 K temperature range, with a collective coupling strength extrapolating to 23 MHz at full polarization. The coupling to multiple modes allows us to distinguish the contributions of dipolar broadening and magnetic field inhomogeneity to the spin linewidth. We find the spin polarization recovery rate to be temperature independent below 1 K and conclude that spin out-diffusion across the resonator mode volume provides the mechanism for spin relaxation of the ensemble. Furthermore, by pumping spins in one sub-ensemble and probing the spins in the other sub-ensembles, we observe fast steady-state cross-relaxation (compared to spin repolarization) across the hyperfine transitions. These observations have important implications for using the three sub-ensembles as independent quantum memories. Research supported by NWO, FOM, and EU Project SOLID

  7. Dynamical Spin Properties of Confined Fermi and Bose Systems in the Presence of Spin-Orbit Coupling

    NASA Astrophysics Data System (ADS)

    Ambrosetti, A.; Salasnich, L.; Silvestrelli, P. L.

    2016-10-01

    Due to the recent experimental progress, tunable spin-orbit (SO) interactions represent ideal candidates for the control of polarization and dynamical spin properties in both quantum wells and cold atomic systems. A detailed understanding of spin properties in SO-coupled systems is thus a compelling prerequisite for possible novel applications or improvements in the context of spintronics and quantum computers. Here, we analyze the case of equal Rashba and Dresselhaus couplings in both homogeneous and laterally confined two-dimensional systems. Starting from the single-particle picture and subsequently introducing two-body interactions we observe that periodic spin fluctuations can be induced and maintained in the system. Through an analytical derivation, we show that the two-body interaction does not involve decoherence effects in the bosonic dimer, and, in the repulsive homogeneous Fermi gas, it may be even exploited in combination with the SO coupling to induce and tune standing currents. By further studying the effects of a harmonic lateral confinement—a particularly interesting case for Bose condensates—we evidence the possible appearance of nontrivial spin textures, whereas the further application of a small Zeeman-type interaction can be exploited to fine-tune the system's polarizability.

  8. Dynamical Spin Properties of Confined Fermi and Bose Systems in the Presence of Spin-Orbit Coupling

    NASA Astrophysics Data System (ADS)

    Ambrosetti, A.; Salasnich, L.; Silvestrelli, P. L.

    2016-04-01

    Due to the recent experimental progress, tunable spin-orbit (SO) interactions represent ideal candidates for the control of polarization and dynamical spin properties in both quantum wells and cold atomic systems. A detailed understanding of spin properties in SO-coupled systems is thus a compelling prerequisite for possible novel applications or improvements in the context of spintronics and quantum computers. Here, we analyze the case of equal Rashba and Dresselhaus couplings in both homogeneous and laterally confined two-dimensional systems. Starting from the single-particle picture and subsequently introducing two-body interactions we observe that periodic spin fluctuations can be induced and maintained in the system. Through an analytical derivation, we show that the two-body interaction does not involve decoherence effects in the bosonic dimer, and, in the repulsive homogeneous Fermi gas, it may be even exploited in combination with the SO coupling to induce and tune standing currents. By further studying the effects of a harmonic lateral confinement—a particularly interesting case for Bose condensates—we evidence the possible appearance of nontrivial spin textures, whereas the further application of a small Zeeman-type interaction can be exploited to fine-tune the system's polarizability.

  9. Spin Texture and Spin Dynamics in Superconducting Cuprates Near the Phase Transition Revealed by the Electron Paramagnetic Resonance

    NASA Astrophysics Data System (ADS)

    Kochelaev, B. I.

    2016-04-01

    A short review of experimental results and theoretical models of the spin texture and spin dynamics in superconducting cuprates near the phase transition developed on the basis of the EPR measurements is given. Distortions of the long-range antiferromagnetic order in the YBa_2 Cu_3 O_{6+y} were investigated for y=0.1-0.4 using Yb^{3+} ions as the EPR probe. In weakly doped samples with y=0.1 , a strong anisotropy of the EPR linewidth is revealed which was related to the indirect spin-spin interaction between the ytterbium ions via antiferromagnetic spin-waves. In the case of the doping level y=0.2-0.3 , the EPR signal consists of narrow and broad lines, which were attributed to formation of charged domain walls. A theoretical analysis is well consistent with experimental results for the case of coplanar elliptical domain walls. A discussion of possible reasons for the observed unusual planar oxygen isotope effect on a critical temperature T_c related to charge heterogeneity in underdoped cuprates is given.

  10. Finite temperature spin-dynamics and phase transitions in spin-orbital models

    SciTech Connect

    Chen, C.-C.

    2010-04-29

    We study finite temperature properties of a generic spin-orbital model relevant to transition metal compounds, having coupled quantum Heisenberg-spin and Ising-orbital degrees of freedom. The model system undergoes a phase transition, consistent with that of a 2D Ising model, to an orbitally ordered state at a temperature set by short-range magnetic order. At low temperatures the orbital degrees of freedom freeze-out and the model maps onto a quantum Heisenberg model. The onset of orbital excitations causes a rapid scrambling of the spin spectral weight away from coherent spin-waves, which leads to a sharp increase in uniform magnetic susceptibility just below the phase transition, reminiscent of the observed behavior in the Fe-pnictide materials.

  11. Spin dynamics of hopping electrons in quantum wires: Algebraic decay and noise

    NASA Astrophysics Data System (ADS)

    Shumilin, A. V.; Sherman, E. Ya.; Glazov, M. M.

    2016-09-01

    We study theoretically the spin decoherence and intrinsic spin noise in semiconductor quantum wires caused by an interplay of electrons hopping between the localized states and the hyperfine interaction of electron and nuclear spins. At a sufficiently low density of localization sites the hopping rates have an exponentially broad distribution. It allows the description of the spin dynamics in terms of closely situated "pairs" of sites and single "reaching" states, from which the series of hops result in electrons localized inside a "pair." The developed analytical model and numerical simulations demonstrate disorder-dependent algebraic tails in the spin decay and power-law singularities features in the low-frequency part of the spin-noise spectrum.

  12. Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3.

    PubMed

    Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S; Tokura, Yoshinori; Nagaosa, Naoto

    2016-01-01

    Weyl fermions that emerge at band crossings in momentum space caused by the spin-orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet. PMID:27273207

  13. Unified dynamics of electrons and photons via Zitterbewegung and spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Leary, C. C.; Smith, Karl H.

    2014-02-01

    We show that when an electron or photon propagates in a cylindrically symmetric waveguide, it experiences both a Zitterbewegung effect and a spin-orbit interaction leading to identical propagation dynamics for both particles. Applying a unified perturbative approach to both particles simultaneously, we find that to first order in perturbation theory, their Hamiltonians each contain identical Darwin (Zitterbewegung) and spin-orbit terms, resulting in the unification of their dynamics. The presence of the Zitterbewegung effect may be interpreted physically as the delocalization of the electron on the scale of its Compton wavelength, or the delocalization of the photon on the scale of its wavelength in the waveguide. The presence of the spin-orbit interaction leads to the prediction of several rotational effects: the spatial or time evolution of either particle's spin or polarization vector is controlled by the sign of its orbital angular momentum quantum number or, conversely, its spatial wave function is controlled by its spin angular momentum.

  14. Spin segregation via dynamically induced long-range interactions in a system of ultracold fermions

    SciTech Connect

    Ebling, Ulrich; Eckardt, Andre; Lewenstein, Maciej

    2011-12-15

    We investigate theoretically the time evolution of a one-dimensional system of spin-1/2 fermions in a harmonic trap after, initially, a spiral spin configuration far from equilibrium is created. We predict a spin segregation building up in time already for weak interaction under realistic experimental conditions. The effect relies on the interplay between exchange interaction and the harmonic trap, and it is found for a wide range of parameters. It can be understood as a consequence of an effective, dynamically induced long-range interaction that is derived by integrating out the rapid oscillatory dynamics in the trap.

  15. SU(2s+1) symmetry and nonlinear dynamics of high spin magnets

    SciTech Connect

    Kovalevsky, M.Y. Glushchenko, A.V.

    2014-10-15

    The article is devoted to the description of dynamics of magnets with arbitrary spin on the basis of the Hamiltonian formalism. The relationship of quantum states and magnetic degrees of freedom has been considered. Subalgebras of Poisson bracket of magnetic values for spin s=1/2; 1; 3/2 have been established. We have obtained non-linear dynamic equations for the normal and degenerate non-equilibrium states of high-spin magnets with the SO(3), SU(4), SU(2)×SU(2), SU(3), SO(4), SO(5) symmetries of exchange interaction. The connection between models of magnetic exchange energy and the Casimir invariants has been discussed.

  16. Entanglement dynamics of spin systems in pure states

    NASA Astrophysics Data System (ADS)

    Furman, G. B.; Meerovich, V. M.; Sokolovsky, V. L.

    2009-09-01

    We investigate numerically the appearance and evolution of entanglement in spin systems prepared initially in a pure state. We consider the dipolar coupling spin systems of different molecular structures: benzene C6H6 , cyclopentane C5H10 , sodium butyrate CH3(CH2)2CO2Na , and calcium hydroxyapatite Ca5(OH)(PO4)3 . Numerical simulations show that the close relationship exists between the intensity of second order (2Q) coherences and concurrences of nearest spins in a cyclopentane molecule.

  17. Modeling two-spin dynamics in a noisy environment

    SciTech Connect

    Testolin, M. J.; Hollenberg, L. C. L.; Cole, J. H.

    2009-10-15

    We describe how the effect of charge noise on a pair of spins coupled via the exchange interaction can be calculated by modeling charge fluctuations as a random telegraph noise process using probability density functions. We develop analytic expressions for the time-dependent superoperator of a pair of spins as a function of fluctuation amplitude and rate. We show that the theory can be extended to include multiple fluctuators, in particular, spectral distributions of fluctuators. These superoperators can be included in time-dependent analyses of the state of spin systems designed for spintronics or quantum information processing to determine the decohering effects of exchange fluctuations.

  18. Dynamic mean field theory of the SK-spin glass. II. Order parameters and gauge invariance

    NASA Astrophysics Data System (ADS)

    Horner, H.

    1984-03-01

    The probability distribution of overlaps proposed by Parisi as order parameter for the SK-spin glass is calculated via dynamics. It is deduced from dynamic response functions and also directly obtained from a treatment with replicas and dynamics. The replica trick is not required. The comparison of the two results shows in which sense fluctuation dissipation theorems hold. Overlaps between three or more states are found to agree with those obtained by Mézard et al. using the replica trick. The origin of the ultrametric topology of spin glass states is investigated within the dynamic mean field theory and a gauge invariance is explored.

  19. Dynamics of an all-optical atomic spin gyroscope.

    PubMed

    Fang, Jiancheng; Wan, Shuangai; Yuan, Heng

    2013-10-20

    We present the transfer function of an all-optical atomic spin gyroscope through a series of differential equations and validate the transfer function by experimental test. A transfer function is the basis for further control system design. We build the differential equations based on a complete set of Bloch equations describing the all-optical atomic spin gyroscope, and obtain the transfer function through application of the Laplace transformation to these differential equations. Moreover, we experimentally validate the transfer function in an all-optical Cs-Xe129 atomic spin gyroscope through a series of step responses. This transfer function is convenient for analysis of the form of control system required. Furthermore, it is available for the design of the control system specifically to improve the performance of all-optical atomic spin gyroscopes.

  20. Atom-diatom scattering dynamics of spinning molecules

    SciTech Connect

    Eyles, C. J.; Floß, J.; Averbukh, I. Sh.; Leibscher, M.

    2015-01-14

    We present full quantum mechanical scattering calculations using spinning molecules as target states for nuclear spin selective atom-diatom scattering of reactive D+H{sub 2} and F+H{sub 2} collisions. Molecules can be forced to rotate uni-directionally by chiral trains of short, non-resonant laser pulses, with different nuclear spin isomers rotating in opposite directions. The calculations we present are based on rotational wavepackets that can be created in this manner. As our simulations show, target molecules with opposite sense of rotation are predominantly scattered in opposite directions, opening routes for spatially and quantum state selective scattering of close chemical species. Moreover, two-dimensional state resolved differential cross sections reveal detailed information about the scattering mechanisms, which can be explained to a large degree by a classical vector model for scattering with spinning molecules.

  1. Entanglement dynamics via geometric phases in quantum spin chains

    SciTech Connect

    Castro, C. S.; Sarandy, M. S.

    2011-04-15

    We introduce a connection between entanglement induced by interaction and geometric phases acquired by a composite quantum spin system. We begin by analyzing the evaluation of cyclic (Aharonov-Anandan) and noncyclic (Mukunda-Simon) geometric phases for general spin chains evolving in the presence of time-independent magnetic fields. Then, by considering Heisenberg chains, we show that the interaction geometric phase, namely, the total geometric phase with subtraction of free spin contributions, is directly related to the global (Meyer-Wallach) entanglement exhibited by an initially separable state during its evolution in Hilbert space. This is analytically shown for N=2 spins and numerically illustrated for larger chains. This relationship promotes the interaction geometric phase to an indicator of global entanglement in the system, which may constitute a useful tool for quantum tasks based on entanglement as a resource to their performance.

  2. Cavity Exciton-Polaritons, Bose Einstein Condensation and Spin Dynamics

    SciTech Connect

    Malpuech, Guillaume; Solnyshkov, Dmitry; Shelykh, Ivan

    2009-10-07

    An introduction giving elementary properties of cavity exciton-polariton will be given. The condition of occurrence of the polariton lasing effect and of the polariton Bose Eintein condensation will be discussed. The impact of the structural disorder on the superfluid behavior of polariton condensates will be analysed. The spin properties of polariton condensates will be discussed. I will show how the anisotropy of the polariton-polariton interaction leads to the suppression of zeeman splitting for polariton condensates (spin Meissner effects). I will show how the combined impact of disorder and spin Meissner effect can lead to the formation of a new condense phase. I will show how these phenomena can allow for the realization of a polaritonic Datta Das spin transistor.

  3. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current

    PubMed Central

    Demidov, V. E.; Evelt, M.; Bessonov, V.; Demokritov, S. O.; Prieto, J. L.; Muñoz, M.; Ben Youssef, J.; Naletov, V. V.; de Loubens, G.; Klein, O.; Collet, M.; Bortolotti, P.; Cros, V.; Anane, A.

    2016-01-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533

  4. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current

    NASA Astrophysics Data System (ADS)

    Demidov, V. E.; Evelt, M.; Bessonov, V.; Demokritov, S. O.; Prieto, J. L.; Muñoz, M.; Ben Youssef, J.; Naletov, V. V.; de Loubens, G.; Klein, O.; Collet, M.; Bortolotti, P.; Cros, V.; Anane, A.

    2016-09-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators.

  5. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current.

    PubMed

    Demidov, V E; Evelt, M; Bessonov, V; Demokritov, S O; Prieto, J L; Muñoz, M; Ben Youssef, J; Naletov, V V; de Loubens, G; Klein, O; Collet, M; Bortolotti, P; Cros, V; Anane, A

    2016-01-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533

  6. Quantum decoherence dynamics of divacancy spins in silicon carbide

    PubMed Central

    Seo, Hosung; Falk, Abram L.; Klimov, Paul V.; Miao, Kevin C.; Galli, Giulia; Awschalom, David D.

    2016-01-01

    Long coherence times are key to the performance of quantum bits (qubits). Here, we experimentally and theoretically show that the Hahn-echo coherence time of electron spins associated with divacancy defects in 4H–SiC reaches 1.3 ms, one of the longest Hahn-echo coherence times of an electron spin in a naturally isotopic crystal. Using a first-principles microscopic quantum-bath model, we find that two factors determine the unusually robust coherence. First, in the presence of moderate magnetic fields (30 mT and above), the 29Si and 13C paramagnetic nuclear spin baths are decoupled. In addition, because SiC is a binary crystal, homo-nuclear spin pairs are both diluted and forbidden from forming strongly coupled, nearest-neighbour spin pairs. Longer neighbour distances result in fewer nuclear spin flip-flops, a less fluctuating intra-crystalline magnetic environment, and thus a longer coherence time. Our results point to polyatomic crystals as promising hosts for coherent qubits in the solid state. PMID:27679936

  7. QUANTUM SIMULATION. Localization-delocalization transition in the dynamics of dipolar-coupled nuclear spins.

    PubMed

    Álvarez, Gonzalo A; Suter, Dieter; Kaiser, Robin

    2015-08-21

    Nonequilibrium dynamics of many-body systems are important in many scientific fields. Here, we report the experimental observation of a phase transition of the quantum coherent dynamics of a three-dimensional many-spin system with dipolar interactions. Using nuclear magnetic resonance (NMR) on a solid-state system of spins at room-temperature, we quench the interaction Hamiltonian to drive the evolution of the system. Depending on the quench strength, we then observe either localized or extended dynamics of the system coherence. We extract the critical exponents for the localized cluster size of correlated spins and diffusion coefficient around the phase transition separating the localized from the delocalized dynamical regime. These results show that NMR techniques are well suited to studying the nonequilibrium dynamics of complex many-body systems. PMID:26293957

  8. All-electrical detection of spin dynamics in magnetic antidot lattices by the inverse spin Hall effect

    NASA Astrophysics Data System (ADS)

    Jungfleisch, Matthias B.; Zhang, Wei; Ding, Junjia; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Hoffmann, Axel

    2016-02-01

    The understanding of spin dynamics in laterally confined structures on sub-micron length scales has become a significant aspect of the development of novel magnetic storage technologies. Numerous ferromagnetic resonance measurements, optical characterization by Kerr microscopy and Brillouin light scattering spectroscopy, and x-ray studies were carried out to detect the dynamics in patterned magnetic antidot lattices. Here, we investigate Oersted-field driven spin dynamics in rectangular Ni80Fe20/Pt antidot lattices with different lattice parameters by electrical means and compare them to micromagnetic simulations. When the system is driven to resonance, a dc voltage across the length of the sample is detected that changes its sign upon field reversal, which is in agreement with a rectification mechanism based on the inverse spin Hall effect. Furthermore, we show that the voltage output scales linearly with the applied microwave drive in the investigated range of powers. Our findings have direct implications on the development of engineered magnonics applications and devices.

  9. Low energy spin dynamics in the spin ice, Ho2Sn2O7

    SciTech Connect

    Ehlers, Georg; Huq, Ashfia; Diallo, Souleymane Omar; Adriano, Cris; Rule, K; Cornelius, A. L.; Fouquet, Peter; Pagliuso, P G; Gardner, Jason

    2012-01-01

    The magnetic properties of Ho{sub 2}Sn{sub 2}O{sub 7} have been investigated and compared to other spin ice compounds. Although the lattice has expanded by 3% relative to the better studied Ho{sub 2}Ti{sub 2}O{sub 7} spin ice, no significant changes were observed in the high temperature properties, T {approx}> 20 K. As the temperature is lowered and correlations develop, Ho{sub 2}Sn{sub 2}O{sub 7} enters its quantum phase at a slightly higher temperature than Ho{sub 2}Ti{sub 2}O{sub 7} and is more antiferromagnetic in character. Below 80 K a weak inelastic mode associated with the holmium nuclear spin system has been measured. The hyperfine field at the holmium nucleus was found to be {approx}700 T.

  10. Molecular Mechanisms of ZnO Nanoparticle Dispersion in Solution: Modeling of Surfactant Association, Electrostatic Shielding and Counter Ion Dynamics

    PubMed Central

    Duchstein, Patrick; Milek, Theodor; Zahn, Dirk

    2015-01-01

    Molecular models of 5 nm sized ZnO/Zn(OH)2 core-shell nanoparticles in ethanolic solution were derived as scale-up models (based on an earlier model created from ion-by-ion aggregation and self-organization) and subjected to mechanistic analyses of surface stabilization by block-copolymers. The latter comprise a poly-methacrylate chain accounting for strong surfactant association to the nanoparticle by hydrogen bonding and salt-bridges. While dangling poly-ethylene oxide chains provide only a limited degree of sterical hindering to nanoparticle agglomeration, the key mechanism of surface stabilization is electrostatic shielding arising from the acrylates and a halo of Na+ counter ions associated to the nanoparticle. Molecular dynamics simulations reveal different solvent shells and distance-dependent mobility of ions and solvent molecules. From this, we provide a molecular rationale of effective particle size, net charge and polarizability of the nanoparticles in solution. PMID:25962096

  11. Molecular Mechanisms of ZnO Nanoparticle Dispersion in Solution: Modeling of Surfactant Association, Electrostatic Shielding and Counter Ion Dynamics.

    PubMed

    Duchstein, Patrick; Milek, Theodor; Zahn, Dirk

    2015-01-01

    Molecular models of 5 nm sized ZnO/Zn(OH)2 core-shell nanoparticles in ethanolic solution were derived as scale-up models (based on an earlier model created from ion-by-ion aggregation and self-organization) and subjected to mechanistic analyses of surface stabilization by block-copolymers. The latter comprise a poly-methacrylate chain accounting for strong surfactant association to the nanoparticle by hydrogen bonding and salt-bridges. While dangling poly-ethylene oxide chains provide only a limited degree of sterical hindering to nanoparticle agglomeration, the key mechanism of surface stabilization is electrostatic shielding arising from the acrylates and a halo of Na+ counter ions associated to the nanoparticle. Molecular dynamics simulations reveal different solvent shells and distance-dependent mobility of ions and solvent molecules. From this, we provide a molecular rationale of effective particle size, net charge and polarizability of the nanoparticles in solution. PMID:25962096

  12. Spin dynamics and Kondo physics in optical tweezers

    NASA Astrophysics Data System (ADS)

    Lin, Yiheng; Lester, Brian J.; Brown, Mark O.; Kaufman, Adam M.; Long, Junling; Ball, Randall J.; Isaev, Leonid; Wall, Michael L.; Rey, Ana Maria; Regal, Cindy A.

    2016-05-01

    We propose to use optical tweezers as a toolset for direct observation of the interplay between quantum statistics, kinetic energy and interactions, and thus implement minimum instances of the Kondo lattice model in systems with few bosonic rubidium atoms. By taking advantage of strong local exchange interactions, our ability to tune the spin-dependent potential shifts between the two wells and complete control over spin and motional degrees of freedom, we design an adiabatic tunneling scheme that efficiently creates a spin-singlet state in one well starting from two initially separated atoms (one atom per tweezer) in opposite spin state. For three atoms in a double-well, two localized in the lowest vibrational mode of each tweezer and one atom in an excited delocalized state, we plan to use similar techniques and observe resonant transfer of two-atom singlet-triplet states between the wells in the regime when the exchange coupling exceeds the mobile atom hopping. Moreover, we argue that such three-atom double-tweezers could potentially be used for quantum computation by encoding logical qubits in collective spin and motional degrees of freedom. Current address: Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.

  13. Dynamics of Polymer Blend Film Formation During Spin Coating

    NASA Astrophysics Data System (ADS)

    Mouhamad, Youmna; Clarke, Nigel; Jones, Richard A. L.; Geoghegan, Mark

    2012-02-01

    Spin casting is a process broadly used to obtain a uniform film on a flat substrate. A homogeneous film results from the balance between centrifugal and viscous forces. Here we revisit the Meyerhofer model of the spin casting process by taking in account the centrifugal forces, a uniform time dependent evaporation rate, and account for the changes in viscosity using the Huggins intrinsic viscosity. Time resolved light reflectometry is used to monitor the thickness changes of a polystyrene-poly(methyl methacrylate)(which we denote as PS and PMMA) film initially dissolved in toluene and spin cast for ten seconds at 1000 rpm. The experimental data are in good agreement with the model. We also investigate how the volume fraction of PS and PMMA influences the thinning of the film during spin casting. A distinct change in the temporal evolution of thickness as a function of time delimits the first phase of the spin casting process where centrifugal forces are dominant from a second phase dominated by the solvent evaporation. This hypothesis is supported by in-situ off specular scattering data. The time at which this change from centrifugal to evaporation-dominated behaviour is delayed as the volume fraction of PMMA increases.

  14. Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO4

    SciTech Connect

    Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas B. S.; Andersen, Niels H.; Li, Jiying; Le, Manh Duc; Laver, Mark; Niedermayer, Christof; Klemke, Bastian; Lefmann, Kim; Vaknin, David

    2015-07-06

    We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c. Furthermore, the possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. While using a spin Hamiltonian, we show that the spin dimensionality is intermediate between XY- and Ising-like, with an easy b axis and a hard c axis. As a result, it is shown that both next-nearest neighbor exchange couplings in the bc plane are in competition with the strongest nearest neighbor coupling.

  15. Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO4

    NASA Astrophysics Data System (ADS)

    Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas B. S.; Andersen, Niels H.; Li, Jiying; Le, Manh Duc; Laver, Mark; Niedermayer, Christof; Klemke, Bastian; Lefmann, Kim; Vaknin, David

    2015-07-01

    We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c . The possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. Using a spin Hamiltonian, we show that the spin dimensionality is intermediate between X Y - and Ising-like, with an easy b axis and a hard c axis. It is shown that both next-nearest neighbor exchange couplings in the b c plane are in competition with the strongest nearest neighbor coupling.

  16. Cascaded spin motive force driven by the dynamics of the skyrmion lattice

    SciTech Connect

    Ohe, Jun-ichiro; Shimada, Yuhki

    2013-12-09

    We numerically investigate the spin motive force (SMF) driven by the dynamics of a Skyrmion lattice. The rotating mode of the Skyrmion core excited by the AC magnetic field induces the large spin-dependent electric field near the core. Due to the collective dynamics of Skyrmion lattice, the measurable voltage is enhanced by the cascade effect of the SMF. The amplitude of the AC voltage is estimated to 30 μV in a macroscopic sample, where 100 Skyrmions exist between two probes. We also investigate the SMF due to the dynamics of the helical magnetic state, where the enhancement of the SMF does not occur.

  17. Effect of surfactant and solvent on spin-lattice relaxation dynamics of magnetic nanocrystals.

    PubMed

    Maiti, Sourav; Chen, Hsiang-Yun; Chen, Tai-Yen; Hsia, Chih-Hao; Son, Dong Hee

    2013-04-25

    The effect of varying the surfactant and solvent medium on the dynamics of spin-lattice relaxation in photoexcited Fe3O4 nanocrystals has been investigated by measuring the time-dependent magnetization employing pump-probe transient Faraday rotation technique. The variation of the surfactants having surface-binding functional groups modified not only the static magnetization but also the dynamics of the recovery of the magnetization occurring via spin-lattice relaxation in the photoexcited Fe3O4 nanocrystals. The variation of the polarity and size of the solvent molecules can also influence the spin-lattice relaxation dynamics. However, the effect is limited to the nanocrystals having sufficiently permeable surfactant layer, where the small solvent molecules (e.g., water) can access the surface and dynamically modify the ligand field on the surface. PMID:23003213

  18. Comparison of quantum and classical relaxation in spin dynamics.

    PubMed

    Wieser, R

    2013-04-01

    The classical Landau-Lifshitz equation with a damping term has been derived from the time evolution of a quantum mechanical wave function under the assumption of a non-Hermitian Hamilton operator. Further, the trajectory of a classical spin (S) has been compared with the expectation value of the spin operator (Ŝ). A good agreement between classical and quantum mechanical trajectories can be found for Hamiltonians linear in Ŝ or S, respectively. Quadratic or higher order terms in the Hamiltonian result in a disagreement.

  19. Dynamic consequences of optical spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Sukhov, Sergey; Kajorndejnukul, Veerachart; Naraghi, Roxana Rezvani; Dogariu, Aristide

    2015-12-01

    Field symmetries and conservation laws are closely associated through Noether's theorem. Light field inhomogeneities lead to changes in linear and angular momenta and, consequently, to radiation pressure, spin or rotation of objects. Here we discuss a new type of mechanical action originating in the exchange between spin and orbital angular momenta. We demonstrate theoretically and experimentally that, when mirror and central symmetries of scattering are broken, a force appears acting perpendicularly to the direction of propagation. This new force completes the set of non-conservative forces (radiation pressure and tractor beams) that can be generated with unstructured light beams.

  20. Spin Crossover in Ferropericlase from First-Principles Molecular Dynamics

    NASA Astrophysics Data System (ADS)

    Holmström, E.; Stixrude, L.

    2015-03-01

    Ferropericlase, (Mg,Fe)O, is the second-most abundant mineral of Earth's lower mantle. With increasing pressure, the Fe ions in the material begin to collapse from a magnetic to nonmagnetic spin state. We present a finite-temperature first-principles phase diagram of this spin crossover, finding a broad pressure range with coexisting magnetic and nonmagnetic ions due to favorable enthalpy of mixing of the two. Furthermore, we find the electrical conductivity of the mineral to reach semimetallic values inside Earth.

  1. Spin crossover in ferropericlase from first-principles molecular dynamics.

    PubMed

    Holmström, E; Stixrude, L

    2015-03-20

    Ferropericlase, (Mg,Fe)O, is the second-most abundant mineral of Earth's lower mantle. With increasing pressure, the Fe ions in the material begin to collapse from a magnetic to nonmagnetic spin state. We present a finite-temperature first-principles phase diagram of this spin crossover, finding a broad pressure range with coexisting magnetic and nonmagnetic ions due to favorable enthalpy of mixing of the two. Furthermore, we find the electrical conductivity of the mineral to reach semimetallic values inside Earth. PMID:25839305

  2. Experimental and theoretical investigation of the magnetization dynamics of an artificial square spin ice cluster

    NASA Astrophysics Data System (ADS)

    Pohlit, Merlin; Stockem, Irina; Porrati, Fabrizio; Huth, Michael; Schröder, Christian; Müller, Jens

    2016-10-01

    We study the magnetization dynamics of a spin ice cluster which is a building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition both experimentally and theoretically. The spin ice cluster is composed of twelve interacting Co nanoislands grown directly on top of a high-resolution micro-Hall sensor. By employing micromagnetic simulations and a macrospin model, we calculate the magnetization and the experimentally investigated stray field emanating from a single nanoisland. The parameters determined from a comparison with the experimental hysteresis loop are used to derive an effective single-dipole macrospin model that allows us to investigate the dynamics of the spin ice cluster. Our model reproduces the experimentally observed non-deterministic sequences in the magnetization curves as well as the distinct temperature dependence of the hysteresis loop.

  3. Dynamical Properties of a Diluted Dipolar-Interaction Heisenberg Spin Glass

    NASA Astrophysics Data System (ADS)

    Zhang, Kai-Cheng; Liu, Yong; Chi, Feng

    2014-02-01

    Up to now the chirality is seldom studied in the diluted spin glass although many investigations have been performed on the site-ordered Edwards—Anderson model. By simulation, we investigate the dynamical properties of both the spin-glass and the chiral-glass phases in a diluted dipolar system, which was manifested to have a spin-glass transition by recent numerical study. By scaling we find that both phases have the same aging behavior and closer aging parameter μ. Similarly, the domains grow in the same way and both phases have a closer barrier exponent Ψ. It means that both the spins and the chirality have the same dynamical properties and they may freeze at the same temperature.

  4. Mean-field dynamics of spin-orbit coupled Bose-Einstein condensates.

    PubMed

    Zhang, Yongping; Mao, Li; Zhang, Chuanwei

    2012-01-20

    Spin-orbit coupling (SOC), the interaction between the spin and momentum of a quantum particle, is crucial for many important condensed matter phenomena. The recent experimental realization of SOC in neutral bosonic cold atoms provides a new and ideal platform for investigating spin-orbit coupled quantum many-body physics. In this Letter, we derive a generic Gross-Pitaevskii equation as the starting point for the study of many-body dynamics in spin-orbit coupled Bose-Einstein condensates. We show that different laser setups for realizing the same SOC may lead to different mean-field dynamics. Various ground state phases (stripe, phase separation, etc.) of the condensate are found in different parameter regions. A new oscillation period induced by the SOC, similar to the Zitterbewegung oscillation, is found in the center-of-mass motion of the condensate.

  5. Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3

    PubMed Central

    Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S.; Tokura, Yoshinori; Nagaosa, Naoto

    2016-01-01

    Weyl fermions that emerge at band crossings in momentum space caused by the spin–orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet. PMID:27273207

  6. Dynamical correlation effects on pair-correlation functions of spin polarized two-dimensional electron gas

    NASA Astrophysics Data System (ADS)

    Kumar, Krishan; Garg, Vinayak; Moudgil, R. K.

    2013-06-01

    We report a theoretical study on the spin-resolved pair-correlation functions gσσ'(r) of a two-dimensional electron gas having arbitrary spin polarization ζ by including the dynamics of exchange-correlations within the dynamical self-consistent mean-field theory of Hasegawa and Shimizu. The calculated g↑↑(r), g↓↓(r) and g↑↓(r) exhibit a nice agreement with the recent quantum Monte Carlo simulation data of Gori-Giorgi et al. However, the agreement for the minority spin correlation function g↓↓(r) decreases with increase in ζ and/or decrease in electron density. Nevertheless, the spin-summed correlation function remains close to the simulation data.

  7. Spin dynamics in patterned nanometer-thick yttrium iron garnet films

    NASA Astrophysics Data System (ADS)

    Jungfleisch, Matthias Benjamin; Zhang, Wei; Jiang, Wanjun; Wu, Stephen M.; Pearson, John E.; Bhattacharya, Anand; Hoffmann, Axel; Sklenar, Joseph; Ketterson, John B.; Chang, Houchen; Wu, Mingzhong

    2015-03-01

    We present experimental investigations on the propagation of spin-wave modes in micro-structured yttrium iron garnet (YIG) stripes.1 The stripes were patterned by photo-lithography from high-quality 40-nm-thick YIG films grown by sputtering.2 Magnetization dynamics is driven by the rf field of a shorted coplanar waveguide patterned onto the YIG stripes. The propagation of spin waves are detected by means of spatially-resolved Brillouin light scattering microscopy. The propagation distance of spin waves is determined in the linear regime, where an exponential decay of 10 μm is observed. The estimated Gilbert damping parameter extracted from the spin-wave decay length is 3 times larger than that obtained through ferromagnetic resonance measurements in unstructured films, which is possibly due to enhanced two-magnon scattering in the patterned films. Furthermore, studies on the spin dynamics driven by spin-torque ferromagnetic resonance in YIG/Pt bilayers and the corresponding spatially-resolved spin-wave distribution are presented. This work was supported by Department of Energy, Office of Science, Materials Science and Engineering Division, the Army Research Office, and National Science Foundation.

  8. Evidence of spin glass dynamics in dilute LiHoxY1-xF4.

    PubMed

    Quilliam, J A; Meng, S; Mugford, C G A; Kycia, J B

    2008-10-31

    ac susceptibility measurements are presented on the dilute, dipolar coupled, Ising magnet LiHoxY1-xF4 for a concentration x=0.045. The frequency and temperature dependences of the susceptibility show characteristic glassy relaxation. The absorption spectrum is found to broaden with decreasing temperature suggesting that the material is behaving as a spin glass and not as an exotic spin liquid as was previously observed. A dynamical scaling analysis suggests a spin glass transition temperature of 43+/-2 mK with an exponent znu=7.8+/-0.2.

  9. Finite-Temperature Entanglement Dynamics in an Anisotropic Two-Qubit Heisenberg Spin Chain

    NASA Astrophysics Data System (ADS)

    Chen, Tao; Shan, Chuanjia; Li, Jinxing; Liu, Tangkun; Huang, Yanxia; Li, Hong

    2010-07-01

    This paper investigates the entanglement dynamics of an anisotropic two-qubit Heisenberg spin chain in the presence of decoherence at finite temperature. The time evolution of the concurrence is studied for different initial Werner states. The influences of initial purity, finite temperature, spontaneous decay and Hamiltonian on the entanglement evolution are analyzed in detail. Our calculations show that the finite temperature restricts the evolution of the entanglement all the time when the Hamiltonian improves it and the spontaneous decay to the reservoirs can produce quantum entanglement with the anisotropy of spin-spin interaction. Finally, the steady-state concurrence which may remain non-zero for low temperature is also given.

  10. Dynamics of spin valves investigated using Magneto-Optical Kerr Effect Spectroscopy

    NASA Astrophysics Data System (ADS)

    Stevens, Christopher; Paul, Jagannath; Dey, Prasenjit; Miller, Casey; McGill, Stephen; Karaiskaj, Denis

    Through an all-optical approach, we are investigating the spin dynamics in different spin torque based structures. Using pump-probe Time-Resolved Magneto-Optical Kerr Effect (TR-MOKE) spectroscopy, we are able to monitor the ultrafast magnon propagation on a sub-picosecond timescale as well as the longer lived oscillations and demagnetization. This represents a recent efforts to realize magnon induced spin torque using an all optical method. This research at USF is supported by the National Science Foundation, Division of Electrical, Communications and Cyber Systems under Grant Number: 1231929. The work was done in part at the NHMFL, Tallahassee, FSU under Grants: DMR-1229217, DMR-1157490.

  11. Modeling Dynamical Black Holes with Spin Parameters Larger Than 0.999

    NASA Astrophysics Data System (ADS)

    Ruchlin, Ian; Etienne, Zachariah

    2016-03-01

    Exploring the extremal Kerr limit in a dynamical, fully general relativistic context may lend insights into the no-hair theorem and uncover new mechanisms by which black hole spins can be increased beyond astrophysical or Kerr limits. Modeling such black holes is highly challenging, with state-of-the-art numerical relativity simulations reaching spin parameters of 0.99 to 0.995 only recently. We have developed new techniques that open the door to stable and reliable puncture black hole evolutions with spin parameters in excess of 0.999. We briefly review these techniques, the results, and possible applications.

  12. The dynamics of particle disks. II - Effects of spin degrees of freedom

    NASA Technical Reports Server (NTRS)

    Araki, Suguru

    1988-01-01

    The present treatment of the thermal equilibria of differentially-rotating, axisymmetric disks consisting of identical, spin-possessing as well as translational DOF-possessing hard sphere particles characterizes these disks' dynamics by means of two novel parameters: (1) the tangential restitution coefficient, and (2) the dimensionless moment of inertia. It is established that rings composed of spinning particles can generally be thermally balanced within more restricted ranges of the optical depth, as well as at higher values of the normal restitution coefficient, than spinless rings. Mean spin is indefinite in the present framework of neglected finite particle-size effects.

  13. Dynamical magnetic anisotropy in spin--1 molecular systems

    NASA Astrophysics Data System (ADS)

    Ruiz-Tijerina, David; Cornaglia, Pablo; Balseiro, Carlos; Ulloa, Sergio

    2012-02-01

    We study electronic transport through a deformable spin-1 molecular system in a break junction setup, under the influence of a local vibrational mode. Our study shows that the magnetic anisotropy, which arises due to stretching along the transport axis[Science 328 1370 (2010)], is renormalized by the interactions with vibrations. The coupling induces additional spin--asymmetric hybridizations that contribute to the net molecular anisotropy. We show that the low temperature physics of such device can be described by an anisotropic Kondo model (J> J), with a magnetic anisotropy term, ANetSz^2, negative at zero stretching. A quantum phase transition (QPT) is explored by stretching the molecule, driving ANet into positive values, and changing the character of the device from a non--Fermi--liquid (NFL) to a Fermi liquid (FL) ground state. This transition can be directly observed through the zero--bias conductance, which we find to be finite for negative anisotropy, zero for positive anisotropy, and to reach the unitary limit at ANet 0. At that point, an underscreened spin-1 Kondo ground state appears due to the restitution of the spin-1 triplet degeneracy.

  14. Existence of a dynamic compensation temperature of the mixed spin-1 and spin-3/2 Ising model within the effective-field theory

    NASA Astrophysics Data System (ADS)

    Shi, Xiaoling; Qi, Yang

    2015-07-01

    The effective-field theory with correlations based on Glauber-type stochastic dynamic is used to study the dynamic compensation behavior of the mixed spin-1 and spin-3/2 ferrimagnetic Ising model. The system is a layered honeycomb structure in which two kinds of spins (spin-1 and spin-3/2) occupy sites alternately. This is related to the experimental works of a molecular-based magnetic multilayer film, AMIIFeII(C2O4)3(A = N(n -CnH 2 n + 1) 4 ,MII = Mn,Fe) . The system is in the presence of a sinusoidal oscillating magnetic field and the Glauber dynamic is used to describe the time evolution of the system. The effects of the interlayer coupling and a crystal-field constant of the spin-1 sublattice on the compensation temperature are investigated. Dynamic phase diagrams, including the compensation points are presented. Besides second-order phase transition, lines of first-order phase transition, the dynamic tricritical point, the dynamic zero-temperature critical point and the multicritical point are found. The dynamic tricritical point, the dynamic compensation point and the non-magnetic phase predicted by the mean-field theory are confirmed by the effective-field theory.

  15. Bed Stability and Debris Flow Erosion: A Dynamic "Shields Criterion" Associated with Bed Structure

    NASA Astrophysics Data System (ADS)

    Longjas, A.; Hill, K. M.

    2015-12-01

    Debris flows are mass movements that play an important role in transporting sediment from steep uplands to rivers at lower slopes. As the debris flow moves downstream, it entrains materials such as loose boulders, gravel, sand and mud deposited locally by shorter flows such as slides and rockfalls. To capture the conditions under which debris flows entrain bed sediment, some models use something akin to the Shields' criterion and an excess shear stress of the flow. However, these models typically neglect granular-scale effects in the bed which can modify the conditions under which a debris flow is erosional or depositional. For example, it is well known that repeated shearing causes denser packing in loose dry soils, which undoubtedly changes their resistance to shear. Here, we present laboratory flume experiments showing that the conditions for entrainment by debris flows is significantly dependent on the aging of an erodible bed even for narrowly distributed spherical particles. We investigate this quantitatively using particle tracking measurements to quantify instantaneous erosion rates and the evolving bed structure or "fabric". With progressive experiments we find a signature that emerges in the bed fabric that is correlated with an increasing apparent "fragility" of the bed. Specifically, a system that is originally depositional may become erosional after repeated debris flow events, and an erodible bed becomes increasingly erodible with repeated flows. We hypothesize that related effects of bed aging at the field scale may be partly responsible for the increasing destructiveness of secondary flows of landslides and debris flows.

  16. Two-level system in spin baths: Non-adiabatic dynamics and heat transport

    SciTech Connect

    Segal, Dvira

    2014-04-28

    We study the non-adiabatic dynamics of a two-state subsystem in a bath of independent spins using the non-interacting blip approximation, and derive an exact analytic expression for the relevant memory kernel. We show that in the thermodynamic limit, when the subsystem-bath coupling is diluted (uniformly) over many (infinite) degrees of freedom, our expression reduces to known results, corresponding to the harmonic bath with an effective, temperature-dependent, spectral density function. We then proceed and study the heat current characteristics in the out-of-equilibrium spin-spin-bath model, with a two-state subsystem bridging two thermal spin-baths of different temperatures. We compare the behavior of this model to the case of a spin connecting boson baths, and demonstrate pronounced qualitative differences between the two models. Specifically, we focus on the development of the thermal diode effect, and show that the spin-spin-bath model cannot support it at weak (subsystem-bath) coupling, while in the intermediate-strong coupling regime its rectifying performance outplays the spin-boson model.

  17. Dynamic nuclear polarization from current-induced electron spin polarization in n-InGaAs

    NASA Astrophysics Data System (ADS)

    Trowbridge, Christopher; Norman, Benjamin; Kato, Yuichiro; Awschalom, David; Sih, Vanessa

    2014-03-01

    Control of the nuclear spin system could prove useful for applications in spintronics or spin-based quantum computation for intermediate term data storage and for the suppression of electron spin dephasing resulting from hyperfine coupling. We investigate the role of nuclear spins in materials with electrically generated spin polarization. The electron spin polarization generated by electrical current in a non-magnetic semiconductor is transferred via dynamic nuclear polarization to the nuclei. The resulting nuclear field is interrogated using Larmor magnetometry. We measure the nuclear field as a function of applied magnetic field, current magnitude and direction, and temperature. An unexpected spatial asymmetry in saturated nuclear field is found. The direction of the nuclear polarization is determined by the directions of the electron spin alignment and external magnetic field, allowing electronic control over the sign of the nuclear alignment direction. Careful study of the nuclear field also enables characterization of the current-induced electron spin polarization in situations that are otherwise experimentally inaccessible. Work supported by AFOSR, NSF and ONR.

  18. Slow Spin Dynamics in Superconducting Ca0.9Ce0.1Fe2As2

    PubMed Central

    Nadeem, K.; Zhang, W.; Chen, D. Y.; Ren, Z. A.; Qiu, X. G.

    2015-01-01

    Slow spin dynamics has been observed in superconducting under-doped Ca0.9Ce0.1Fe2As2 single crystal. Below 100 K, the system exhibits hysteresis in the cooling and warming protocols of temperature dependent resistivity due to first order tetragonal to orthorhombic structural transition with simultaneous magnetic transition from paramagnetic to spin density wave antiferromagnetic state of the iron (Fe) ions. Zero field cooled/field cooled (ZFC/FC) magnetization curves showed splitting at 32 K followed by a sharp increase of the FC curve and then FC plateau at low temperatures. Slow spin relaxation in both the ZFC and FC protocols was observed which is typical for spin-glass system. The system also showed features analogue to spin-glass behavior such as ZFC peak, FC plateau, ZFC slow spin relaxation, magnetic hysteresis, and ZFC ac memory effect. The spin-glass like behavior was rather weak and vanished at higher fields. The origin of the slow spin dynamics could be the inhomogeneous distribution of the cerium (Ce) spins ordered along the c-axis OR interactions between Fe and Ce spins which lead to magnetic frustration of Ce spins. All these findings support the coexistence of slow spin dynamics of Ce spins and superconductivity in Ca0.9Ce0.1Fe2As2 single crystal. PMID:26024047

  19. Scalar relaxation of the second kind - a potential source of information on the dynamics of molecular movements. 2. Magnetic dipole moments and magnetic shielding of bromine nuclei.

    PubMed

    Gryff-Keller, Adam; Molchanov, Sergey; Wodyński, Artur

    2014-01-01

    In this paper, we continue the exploration of possibilities, limitations, and methodological problems of the studies based on measurements of the nuclear spin relaxation rates running via the scalar relaxation of the second kind (SC2) mechanism. The attention has been focused on the (13)C-(79)Br and (13)C-(81)Br systems in organic bromo compounds, which are characterized by exceptionally small differences of Larmor frequencies, ΔωCBr, of the coupled nuclei. This unique property enables experimental observation of longitudinal SC2 relaxation of (13)C nuclei, which makes investigation of the SC2 relaxation rates an attractive experimental method of determination of spin-spin coupling constants and relaxation rates of quadrupole bromine nuclei, both types of parameters being hardly accessible by direct measurements. A careful examination of the methodology used in SC2 relaxation studies of carbon-bromine systems reveals, however, some disturbing facts that could burden the results with systematic inaccuracies. Namely, the way of calculating the Larmor frequency differences between (13)C and bromine isotopes, ΔωCBr, may cause some reservations. In this work, the values of (79)Br and (81)Br magnetogyric ratios have been rechecked using bromine NMR data for the KBr·Kryptofix 222 complex in acetonitrile solution and the results of the advanced calculations of the magnetic shielding of the bromine nucleus in the Br(-) anion. Moreover, it has been pointed out that in the case of (13)C-(79)Br, the magnetic shielding of the bromine nucleus in the investigated molecule must not be neglected during the calculation of the ΔωCBr parameter. Some recommendations concerning the exploitation of available theoretical methods to calculate bromine shielding constants for bromo compounds have also been formulated, keeping in mind relativistic effects.

  20. Spin dynamics in SiGe quantum dot lines and ring molecules

    NASA Astrophysics Data System (ADS)

    Zinovieva, A. F.; Nenashev, A. V.; Dvurechenskii, A. V.

    2016-04-01

    Semiconductor quantum dot (QD) structures can be used as a model for understanding the effect of the microscopic structure, symmetry of crystals, and molecules on their macroscopic properties. In this work, the results of two theoretical approaches demonstrate that the spin dynamics in ordered QD structures depends on the size, spatial configuration, and topology of the object built of QDs. It was shown that the spin dynamics in QD structures with the hopping regime of conductivity significantly differs from the spin dynamics in two-dimensional (2D) and three-dimensional (3D) structures being at the other side of the metal-insulator transition. The special character of the effective magnetic field δ H fluctuations appearing only during tunneling between quantum dots is responsible for the insensitivity of spin relaxation times to the magnitude of the external magnetic field in infinite QD structures (2D square lattice and 1D linear QD chain). In finite QD structures (QD rings and linear chains), an external magnetic field H0 is directly involved in the spin relaxation process and spin is lost due to interaction with a special combination of fields Δ H ˜[H0×δ H ]/δ H that leads to an unusual orientation dependence of ESR linewidth, recently observed for QD chains. It was shown that the ordering of QD structures can be used for the conservation of spin orientation. For 1D finite quantum dot chains, the ordering can provide the stabilization of all spin components Sx,Sy, and Sz, while for ringlike molecules only Sz polarization can be stabilized. The results obtained in this work can be useful for development of novel semiconductor devices and in quantum information processing.

  1. Dynamic stability of a spinning tube conveying a fluid through a symmetrical noncircular cross-section

    SciTech Connect

    Benedetti, G.A.

    1990-11-01

    When a fluid flows inside a tube, the deformations of the tube can interact with the fluid flowing within it and these dynamic interactions can result in significant lateral motions of the tube and the flowing fluid. The purpose of this report is to examine the dynamic stability of a spinning tube through which an incompressible frictionless fluid is flowing. The tube can be considered as either a hollow beam or a hollow cable. The analytical results can be applied to spinning or stationary tubes through which fluids are transferred; e.g., liquid coolants, fuels and lubricants, slurry solutions, and high explosives in paste form. The coupled partial differential equations are determined for the lateral motion of a spinning Bernoulli-Euler beam or a spinning cable carrying an incompressible flowing fluid. The beam, which spins about an axis parallel to its longitudinal axis and which can also be loaded by a constant axial force, is straight, uniform, simply supported, and rests on a massless, uniform elastic foundation that spins with the beam. Damping for the beam and foundation is considered by using a combined uniform viscous damping coefficient. The fluid, in addition to being incompressible, is frictionless, has a constant density, and flows at a constant speed relative to the longitudinal beam axis. The Galerkin method is used to reduce the coupled partial differential equations for the lateral motion of the spinning beam to a coupled set of 2N, second order, ordinary differential equations for the generalized beam coordinates. By simplifying these equations and examining the roots of the characteristic equation, an analytical solution is obtained for the lateral dynamic instability of the beam (or cable). The analytical solutions determined the minimum critical fluid speed and the critical spin speeds, for a specified fluid speed, in terms of the physical parameters of the system.

  2. Effect of modularity on the Glauber dynamics of the dilute spin glass model

    NASA Astrophysics Data System (ADS)

    Park, Jeong-Man

    2014-11-01

    We study the Glauber dynamics of the dilute, infinite-ranged spin glass model, the so-called dilute Sherrington-Kirkpatrick (dSK) model. The dSK model has sparse couplings and can be classified by the modularity ( M) of the coupling matrix. We investigate the effect of the modularity on the relaxation dynamics starting from a random initial state. By using the Glauber dynamics and the replica method, we derive the relaxation dynamics equations for the magnetization ( m) and the energy per spin ( r), in addition to the equation for the spin glass order parameter ( q αβ ). In the replica symmetric (RS) analysis, we find that there are two solutions for the RS spin glass order parameter ( q): q = 0which is stable for r < 1/2 and q = (-1+4 r 2)/(32 r 4) which is stable for r > 1/2 in the non-modular system and q = 0 which is stable for r < 1/ and q = (-1+8 r 2)/(128 r 4) which is stable for r > 1/ in the completely modular system. By substituting the proper q values into the equations for r, we find that the relaxation dynamics of r depends on the modularity, M. These results suggest that, in the context of evolutionary theory, the modularity may emerge spontaneously in the point-mutation-only framework (Glauber dynamics) under a changing environment.

  3. Flight dynamics of a spinning projectile descending on a parachute

    SciTech Connect

    Benedetti, G.A.

    1989-02-01

    During the past twenty years Sandia National Laboratories and the US Army have vertically gun launched numerous 155mm and eight-inch diameter flight test projectiles. These projectiles are subsequently recovered using an on-board parachute recovery system which is attached to the forward case structure of the projectile. There have been at least five attempts to describe, through analytical and numerical simulations, the translational and rotational motions of a spinning projectile descending on a parachute. However, none of these investigations have correctly described the large nutational motion of the projectile since all of them overlooked the fundamental mechanism which causes these angular motions. Numerical simulations as well as a closed form analytical solution show conclusively that the Magnus moment is responsible for the large nutational motion of the projectile. That is, when the center of pressure for the Magnus force is aft of the center of mass for the projectile, the Magnus moment causes an unstable (or large) nutational motion which always tends to turn the spinning projectile upside down while it is descending on the parachute. Conversely, when the center of mass for the projectile is aft of the center of pressure for the Magnus force, the Magnus moment stabilizes the nutational motion tending to always point the base of the spinning projectile down. The results of this work are utilized to render projectile parachute recovery systems more reliable and to explain what initially may appear to be strange gyrodynamic behavior of a spinning projectile descending on a parachute. 14 refs., 20 figs.

  4. Attitude dynamic of spin-stabilized satellites with flexible appendages

    NASA Technical Reports Server (NTRS)

    Renard, M. L.

    1973-01-01

    Equations of motion and computer programs have been developed for analyzing the motion of a spin-stabilized spacecraft having long, flexible appendages. Stability charts were derived, or can be redrawn with the desired accuracy for any particular set of design parameters. Simulation graphs of variables of interest are readily obtainable on line using program FLEXAT. Finally, applications to actual satellites, such as UK-4 and IMP-1 have been considered.

  5. Spin dynamics in the frozen state of the dipolar spin ice material Dy2Ti2O7

    NASA Astrophysics Data System (ADS)

    Yaraskavitch, L. R.; Revell, H. M.; Meng, S.; Ross, K. A.; Noad, H. M. L.; Dabkowska, H. A.; Gaulin, B. D.; Kycia, J. B.

    2012-01-01

    Low-temperature magnetic ac susceptibility measurements of single-crystal dipolar spin ice Dy2Ti2O7 are presented. The relaxation is found to exhibit thermally activated Arrhenius behavior with an activation energy of 9.79 K (˜9Jeff), which is not consistent with a simple scaling of 6Jeff, as previously found for Ho2Ti2O7. There are distinct quantifiable differences between Dy2Ti2O7 and Ho2Ti2O7 absorption spectra. The measured dynamics does not agree with simulations based on current magnetic monopole theory nor thermal relaxation measurements, but instead freezes out at a faster rate.

  6. SPILADY: A parallel CPU and GPU code for spin-lattice magnetic molecular dynamics simulations

    NASA Astrophysics Data System (ADS)

    Ma, Pui-Wai; Dudarev, S. L.; Woo, C. H.

    2016-10-01

    Spin-lattice dynamics generalizes molecular dynamics to magnetic materials, where dynamic variables describing an evolving atomic system include not only coordinates and velocities of atoms but also directions and magnitudes of atomic magnetic moments (spins). Spin-lattice dynamics simulates the collective time evolution of spins and atoms, taking into account the effect of non-collinear magnetism on interatomic forces. Applications of the method include atomistic models for defects, dislocations and surfaces in magnetic materials, thermally activated diffusion of defects, magnetic phase transitions, and various magnetic and lattice relaxation phenomena. Spin-lattice dynamics retains all the capabilities of molecular dynamics, adding to them the treatment of non-collinear magnetic degrees of freedom. The spin-lattice dynamics time integration algorithm uses symplectic Suzuki-Trotter decomposition of atomic coordinate, velocity and spin evolution operators, and delivers highly accurate numerical solutions of dynamic evolution equations over extended intervals of time. The code is parallelized in coordinate and spin spaces, and is written in OpenMP C/C++ for CPU and in CUDA C/C++ for Nvidia GPU implementations. Temperatures of atoms and spins are controlled by Langevin thermostats. Conduction electrons are treated by coupling the discrete spin-lattice dynamics equations for atoms and spins to the heat transfer equation for the electrons. Worked examples include simulations of thermalization of ferromagnetic bcc iron, the dynamics of laser pulse demagnetization, and collision cascades. Catalogue identifier: AFAN_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AFAN_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: Apache License, Version 2.0 No. of lines in distributed program, including test data, etc.: 1611165 No. of bytes in distributed program, including test data, etc.: 367246683

  7. RosettaEPR: Rotamer Library for Spin Label Structure and Dynamics

    PubMed Central

    Alexander, Nathan S.; Stein, Richard A.; Koteiche, Hanane A.; Kaufmann, Kristian W.; Mchaourab, Hassane S.; Meiler, Jens

    2013-01-01

    An increasingly used parameter in structural biology is the measurement of distances between spin labels bound to a protein. One limitation to these measurements is the unknown position of the spin label relative to the protein backbone. To overcome this drawback, we introduce a rotamer library of the methanethiosulfonate spin label (MTSSL) into the protein modeling program Rosetta. Spin label rotamers were derived from conformations observed in crystal structures of spin labeled T4 lysozyme and previously published molecular dynamics simulations. Rosetta’s ability to accurately recover spin label conformations and EPR measured distance distributions was evaluated against 19 experimentally determined MTSSL labeled structures of T4 lysozyme and the membrane protein LeuT and 73 distance distributions from T4 lysozyme and the membrane protein MsbA. For a site in the core of T4 lysozyme, the correct spin label conformation (Χ1 and Χ2) is recovered in 99.8% of trials. In surface positions 53% of the trajectories agree with crystallized conformations in Χ1 and Χ2. This level of recovery is on par with Rosetta performance for the 20 natural amino acids. In addition, Rosetta predicts the distance between two spin labels with a mean error of 4.4 Å. The width of the experimental distance distribution, which reflects the flexibility of the two spin labels, is predicted with a mean error of 1.3 Å. RosettaEPR makes full-atom spin label modeling available to a wide scientific community in conjunction with the powerful suite of modeling methods within Rosetta. PMID:24039810

  8. Geometric phases and quantum correlations dynamics in spin-boson model

    SciTech Connect

    Wu, Wei; Xu, Jing-Bo

    2014-01-28

    We explore the dynamics of spin-boson model for the Ohmic bath by employing the master equation approach and obtain an explicit expression of reduced density matrix. We also calculate the geometric phases of the spin-boson model by making use of the analytical results and discuss how the dissipative bosonic environment affects geometric phases. Furthermore, we investigate the dynamics of quantum discord and entanglement of two qubits each locally interacting with its own independent bosonic environments. It is found that the decay properties of quantum discord and entanglement are sensitive to the choice of initial state's parameter and coupling strength between system and bath.

  9. A spin-wave logic gate based on a width-modulated dynamic magnonic crystal

    SciTech Connect

    Nikitin, Andrey A.; Ustinov, Alexey B.; Semenov, Alexander A.; Kalinikos, Boris A.; Chumak, Andrii V.; Serga, Alexander A.; Vasyuchka, Vitaliy I.; Hillebrands, Burkard; Lähderanta, Erkki

    2015-03-09

    An electric current controlled spin-wave logic gate based on a width-modulated dynamic magnonic crystal is realized. The device utilizes a spin-wave waveguide fabricated from a single-crystal Yttrium Iron Garnet film and two conducting wires attached to the film surface. Application of electric currents to the wires provides a means for dynamic control of the effective geometry of waveguide and results in a suppression of the magnonic band gap. The performance of the magnonic crystal as an AND logic gate is demonstrated.

  10. Effect of thermal fluctuations in spin-torque driven magnetization dynamics

    NASA Astrophysics Data System (ADS)

    Bonin, R.; Bertotti, G.; Serpico, C.; Mayergoyz, I. D.; d'Aquino, M.

    2007-09-01

    Nanomagnets with uniaxial symmetry driven by an external field and spin-polarized currents are considered. Anisotropy, applied field, and spin polarization are all aligned along the symmetry axis. Thermal fluctuations are described by adding a Gaussian white noise stochastic term to the Landau-Lifshitz-Gilbert equation for the deterministic dynamics. The corresponding Fokker-Planck equation is derived. It is shown that deterministic dynamics, thermal relaxation, and transition rate between stable states are governed by an effective potential including the effect of current injection.

  11. Lattice Dynamics of EuO: Evidence for Giant Spin-Phonon Coupling.

    PubMed

    Pradip, R; Piekarz, P; Bosak, A; Merkel, D G; Waller, O; Seiler, A; Chumakov, A I; Rüffer, R; Oleś, A M; Parlinski, K; Krisch, M; Baumbach, T; Stankov, S

    2016-05-01

    Comprehensive studies of lattice dynamics in the ferromagnetic semiconductor EuO have been performed by a combination of inelastic x-ray scattering, nuclear inelastic scattering, and ab initio calculations. A remarkably large broadening of the transverse acoustic phonons was discovered at temperatures above and below the Curie temperature T_{C}=69  K. This result indicates a surprisingly strong momentum-dependent spin-phonon coupling induced by the spin dynamics in EuO. PMID:27203332

  12. Non-local detection of spin dynamics via spin rectification effect in yttrium iron garnet/SiO{sub 2}/NiFe trilayers near simultaneous ferromagnetic resonance

    SciTech Connect

    Soh, Wee Tee Ong, C. K.; Peng, Bin

    2015-08-15

    The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO{sub 2} spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.

  13. Dynamics and control of flexible spinning solar sails under reflectivity modulation

    NASA Astrophysics Data System (ADS)

    Mu, Junshan; Gong, Shengping; Ma, Pengbin; Li, Junfeng

    2015-10-01

    Electrochromic devices have been used for the attitude control of a spinning solar sail in a deep space mission by modulating the reflectivity of the sail membrane. As a flexible spinning solar sail has no rigid structure to support its membrane, the distributed load due to solar radiation will lead to the deformation of the sail membrane, and the control torque generated by reflectivity modulation can introduce oscillatory motion to the membrane. By contrast, the deformation and oscillatory motion of the sail membrane have an impact on the performance of the reflectivity control. This paper investigates the dynamics and control of flexible spinning solar sails under reflectivity modulation. The static deformation of a spinning sail membrane subjected to solar radiation pressure in an equilibrium state is analyzed. The von Karman theory is used to obtain the displacements and the stress distribution in the equilibrium states. A simplified analytical first-order mode is chosen to model the membrane oscillation. The coupled membrane oscillation-attitude-orbit dynamics are considered for a GeoSail formation flying mission. The relative attitude and orbit control of flexible spinning solar sails under reflectivity modulation are numerically tested. The simulations indicate that the membrane deformation and oscillation have a lower impact on the control of the reflectivity modulated sails than the increase of the spinning rate.

  14. Spin dynamics of the ordered dipolar-octupolar pseudospin-1/2 pyrochlore Nd2Zr2O7 probed by muon spin relaxation

    NASA Astrophysics Data System (ADS)

    Xu, J.; Balz, C.; Baines, C.; Luetkens, H.; Lake, B.

    2016-08-01

    We present a muon spin relaxation study on the Ising pyrochlore Nd2Zr2O7 which develops an "all-in-all-out" magnetic order below 0.4 K. At 20 mK, far below the ordering transition temperature, the zero-field muon spin relaxation spectra show no static features and can be well described by a dynamical Gaussian-broadened Gaussian Kubo-Toyabe function indicating strong fluctuations of the ordered state. The spectra of the paramagnetic state (below 4.2 K) reveal anomalously slow paramagnetic spin dynamics and show only a small difference with the spectra of the ordered state. We find that the fluctuation rate decreases with decreasing temperature and becomes nearly temperature independent below the transition temperature, indicating persistent slow spin dynamics in the ground state. The field distribution width shows a small but sudden increase at the transition temperature and then becomes almost constant. The spectra in applied longitudinal fields are well fitted by the conventional dynamical Gaussian Kubo-Toyabe function, which further supports the dynamical nature of the ground state. The fluctuation rate shows a peak as a function of external field which is associated with a field-induced spin-flip transition. The strong dynamics in the ordered state is attributed to the transverse coupling of the Ising spins introduced by the multipole interactions.

  15. Hyperfine and spin-orbit dynamics in GaAs double quantum dots

    NASA Astrophysics Data System (ADS)

    Shulman, Michael; Nichol, John; Harvey, Shannon; Pal, Arijeet; Halperin, Bertrand; Umansky, Vladimir; Yacoby, Amir

    2015-03-01

    Semiconductor quantum dots provide a unique platform for single-particle physics and many-body quantum mechanics. In particular, understanding the dynamics of a single electron interacting with a nuclear spin bath is key to improving spin-based quantum information processing, since the hyperfine interaction limits the performance of many spin qubits. We probe the electron-nuclear interaction by measuring the splitting at the anti-crossing between the electron singlet (S) and m =1 triplet (T +) states in a GaAs double quantum dot. Using Landau-Zener sweeps, we find that the size of this splitting varies by more than an order of magnitude depending on the magnitude and direction of the external magnetic field. These results are consistent with a competition between the spin orbit interaction and the hyperfine interaction, even though the extracted spin orbit length is much larger than the size of the double quantum dot. We confirm these results by using Landau-Zener sweeps to measure the high-frequency correlations in the S-T + splitting that arise from the Larmor precession of the nuclei. These unexpected results have implications for improving the performance of spin-based quantum information processing, as well as improving our understanding of the central spin problem.

  16. Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes

    NASA Astrophysics Data System (ADS)

    Mi, Bin-Zhou

    2016-09-01

    The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green's function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.

  17. Dynamic properties of magnets with spin S = 3/2 and non-Heisenberg isotropic interaction

    SciTech Connect

    Kosmachev, O. A.; Fridman, Yu. A.; Galkina, E. G.; Ivanov, B. A.

    2015-02-15

    The dynamic properties of a magnet with magnetic-ion spin of 3/2 and an isotropic spin interaction of a general form have been investigated. Only four phase states can be realized in the system under consideration at various relationships between the material parameters: the ferro- and antiferromagnetic phases with saturated spin and the states with tensor order parameters, the nematic and antinematic ones. For these phases, the spontaneous symmetry breaking is determined by the octupole order parameter containing the mean values trilinear in spin operator components at a given site. The spectra of elementary excitations have been determined in all phases. Additional branches of excitations arise in all four phase states.

  18. The magnetic field dependence of cross-effect dynamic nuclear polarization under magic angle spinning

    SciTech Connect

    Mance, Deni; Baldus, Marc; Gast, Peter; Huber, Martina; Ivanov, Konstantin L.

    2015-06-21

    We develop a theoretical description of Dynamic Nuclear Polarization (DNP) in solids under Magic Angle Spinning (MAS) to describe the magnetic field dependence of the DNP effect. The treatment is based on an efficient scheme for numerical solution of the Liouville-von Neumann equation, which explicitly takes into account the variation of magnetic interactions during the sample spinning. The dependence of the cross-effect MAS-DNP on various parameters, such as the hyperfine interaction, electron-electron dipolar interaction, microwave field strength, and electron spin relaxation rates, is analyzed. Electron spin relaxation rates are determined by electron paramagnetic resonance measurements, and calculations are compared to experimental data. Our results suggest that the observed nuclear magnetic resonance signal enhancements provided by MAS-DNP can be explained by discriminating between “bulk” and “core” nuclei and by taking into account the slow DNP build-up rate for the bulk nuclei.

  19. Low field domain wall dynamics in artificial spin-ice basis structure

    SciTech Connect

    Kwon, J.; Goolaup, S.; Lim, G. J.; Kerk, I. S.; Lew, W. S.; Chang, C. H.; Roy, K.

    2015-10-28

    Artificial magnetic spin-ice nanostructures provide an ideal platform for the observation of magnetic monopoles. The formation of a magnetic monopole is governed by the motion of a magnetic charge carrier via the propagation of domain walls (DWs) in a lattice. To date, most experiments have been on the static visualization of DW propagation in the lattice. In this paper, we report on the low field dynamics of DW in a unit spin-ice structure measured by magnetoresistance changes. Our results show that reversible DW propagation can be initiated within the spin-ice basis. The initial magnetization configuration of the unit structure strongly influences the direction of DW motion in the branches. Single or multiple domain wall nucleation can be induced in the respective branches of the unit spin ice by the direction of the applied field.

  20. Chaotic dynamics of stellar spin in binaries and the production of misaligned hot Jupiters.

    PubMed

    Storch, Natalia I; Anderson, Kassandra R; Lai, Dong

    2014-09-12

    Many exoplanetary systems containing hot Jupiters are observed to have highly misaligned orbital axes relative to the stellar spin axes. Kozai-Lidov oscillations of orbital eccentricity and inclination induced by a binary companion, in conjunction with tidal dissipation, constitute a major channel for the production of hot Jupiters. We demonstrate that gravitational interaction between the planet and its oblate host star can lead to chaotic evolution of the stellar spin axis during Kozai cycles. As parameters such as the planet mass and stellar rotation period are varied, periodic islands can appear in an ocean of chaos, in a manner reminiscent of other dynamical systems. In the presence of tidal dissipation, the complex spin evolution can leave an imprint on the final spin-orbit misalignment angles. PMID:25214623

  1. Chaotic dynamics of stellar spin in binaries and the production of misaligned hot Jupiters.

    PubMed

    Storch, Natalia I; Anderson, Kassandra R; Lai, Dong

    2014-09-12

    Many exoplanetary systems containing hot Jupiters are observed to have highly misaligned orbital axes relative to the stellar spin axes. Kozai-Lidov oscillations of orbital eccentricity and inclination induced by a binary companion, in conjunction with tidal dissipation, constitute a major channel for the production of hot Jupiters. We demonstrate that gravitational interaction between the planet and its oblate host star can lead to chaotic evolution of the stellar spin axis during Kozai cycles. As parameters such as the planet mass and stellar rotation period are varied, periodic islands can appear in an ocean of chaos, in a manner reminiscent of other dynamical systems. In the presence of tidal dissipation, the complex spin evolution can leave an imprint on the final spin-orbit misalignment angles.

  2. EPR, charge transport, and spin dynamics in doped polyanilines

    NASA Astrophysics Data System (ADS)

    Kon'kin, A. L.; Shtyrlin, V. G.; Garipov, R. R.; Aganov, A. V.; Zakharov, A. V.; Krinichnyi, V. I.; Adams, P. N.; Monkman, A. P.

    2002-08-01

    Charge transport and magnetic properties of films of polyaniline (PAN) doped with 10-camphorsulfonic acid and 2-acrylamido-2-methyl-1-propanesulfonic acid (AMPSA) have been studied by conductivity, magnetic-susceptibility superconducting quantum interference device measurements, and 3-cm and 8-mm electron paramagnetic resonance (EPR) spectroscopy at doping levels (x) from 0.3 to 0.9 over a temperature range from 15 to 300 K. The temperature dependences of conductivities were explained in terms of the advanced multiphase heterogeneous granular metallic (HGM) model with percolation including disordered metallic (DM) and nonmetallic (NM) phases. The anomalous conductivity change in the PAN-AMPSAx system at T>240 K was accounted quantitatively for a solid-phase equilibrium with the occurrence of the disordered anion phase from the metallic islands. A means for analysis of the EPR line shape in conducting media has been developed and, with this, conductivity and microwave dielectric constants were estimated and two EPR signals, R1 and R2, were detected in both systems. It was shown that R1 signal belongs to pinned radicals of isolated polymer chains, whereas R2 is the weight-averaged signal, resulting from three types of paramagnetic centers, localized and mobile spins in the NM and DM phases, which interact via exchange. From the temperature and frequency dependences of the R2 linewidth the spin-diffusion parameters for the NM phase in both systems were determined. It was found that the HGM model allows good explanation of both charge transport and spin diffusion in the doped polyaniline films.

  3. Kinetic theories for spin models for cooperative relaxation dynamics

    NASA Astrophysics Data System (ADS)

    Pitts, Steven Jerome

    The facilitated kinetic Ising models with asymmetric spin flip constraints introduced by Jackle and co-workers [J. Jackle, S. Eisinger, Z. Phys. B 84, 115 (1991); J. Reiter, F. Mauch, J. Jackle, Physica A 184, 458 (1992)] exhibit complex relaxation behavior in their associated spin density time correlation functions. This includes the growth of relaxation times over many orders of magnitude when the thermodynamic control parameter is varied, and, in some cases, ergodic-nonergodic transitions. Relaxation equations for the time dependence of the spin density autocorrelation function for a set of these models are developed that relate this autocorrelation function to the irreducible memory function of Kawasaki [K. Kawasaki, Physica A 215, 61 (1995)] using a novel diagrammatic series approach. It is shown that the irreducible memory function in a theory of the relaxation of an autocorrelation function in a Markov model with detailed balance plays the same role as the part of the memory function approximated by a polynomial function of the autocorrelation function with positive coefficients in schematic simple mode coupling theories for supercooled liquids [W. Gotze, in Liquids, Freezing and the Glass Transition, D. Levesque, J. P. Hansen, J. Zinn-Justin eds., 287 (North Holland, New York, 1991)]. Sets of diagrams in the series for the irreducible memory function are summed which lead to approximations of this type. The behavior of these approximations is compared with known results from previous analytical calculations and from numerical simulations. For the simplest one dimensional model, relaxation equations that are closely related to schematic extended mode coupling theories [W. Gotze, ibid] are also derived using the diagrammatic series. Comparison of the results of these approximate theories with simulation data shows that these theories improve significantly on the results of the theories of the simple schematic mode coupling theory type. The potential

  4. Distinguishing the ultrafast dynamics of spin and orbital moments in solids.

    PubMed

    Boeglin, C; Beaurepaire, E; Halté, V; López-Flores, V; Stamm, C; Pontius, N; Dürr, H A; Bigot, J-Y

    2010-05-27

    For an isolated quantum particle, such as an electron, the orbital (L) and spin (S) magnetic moments can change provided that the total angular momentum of the particle is conserved. In condensed matter, an efficient transfer between L and S can occur owing to the spin-orbit interaction, which originates in the relativistic motion of electrons. Disentangling the absolute contributions of the orbital and spin angular momenta is challenging, however, as any transfer between the two occurs on femtosecond timescales. Here we investigate such phenomena by using ultrashort optical laser pulses to change the magnetization of a ferromagnetic film and then probe its dynamics with circularly polarized femtosecond X-ray pulses. Our measurements enable us to disentangle the spin and orbital components of the magnetic moment, revealing different dynamics for L and S. We highlight the important role played by the spin-orbit interaction in the ultrafast laser-induced demagnetization of ferromagnetic films, and show also that the magneto-crystalline anisotropy energy is an important quantity to consider in such processes. Our study provides insights into the dynamics in magnetic systems as well as perspectives for the ultrafast control of information in magnetic recording media.

  5. Non-Markovian dynamics in chiral quantum networks with spins and photons

    NASA Astrophysics Data System (ADS)

    Ramos, Tomás; Vermersch, Benoît; Hauke, Philipp; Pichler, Hannes; Zoller, Peter

    2016-06-01

    We study the dynamics of chiral quantum networks consisting of nodes coupled by unidirectional or asymmetric bidirectional quantum channels. In contrast to familiar photonic networks where driven two-level atoms exchange photons via 1D photonic nanostructures, we propose and study a setup where interactions between the atoms are mediated by spin excitations (magnons) in 1D X X spin chains representing spin waveguides. While Markovian quantum network theory eliminates quantum channels as structureless reservoirs in a Born-Markov approximation to obtain a master equation for the nodes, we are interested in non-Markovian dynamics. This arises from the nonlinear character of the dispersion with band-edge effects, and from finite spin propagation velocities leading to time delays in interactions. To account for the non-Markovian dynamics we treat the quantum degrees of freedom of the nodes and connecting channel as a composite spin system with the surrounding of the quantum network as a Markovian bath, allowing for an efficient solution with time-dependent density matrix renormalization-group techniques. We illustrate our approach showing non-Markovian effects in the driven-dissipative formation of quantum dimers, and we present examples for quantum information protocols involving quantum state transfer with engineered elements as basic building blocks of quantum spintronic circuits.

  6. Modular shield

    DOEpatents

    Snyder, Keith W.

    2002-01-01

    A modular system for containing projectiles has a sheet of material including at least a polycarbonate layer held by a metal frame having a straight frame member corresponding to each straight edge of the sheet. Each frame member has a U-shaped shield channel covering and holding a straight edge of the sheet and an adjacent U-shaped clamp channel rigidly held against the shield channel. A flexible gasket separates each sheet edge from its respective shield channel; and each frame member is fastened to each adjacent frame member only by clamps extending between adjacent clamp channels.

  7. Dynamics of polymer film formation during spin coating

    SciTech Connect

    Mouhamad, Y.; Clarke, N.; Jones, R. A. L.; Geoghegan, M.; Mokarian-Tabari, P.

    2014-09-28

    Standard models explaining the spin coating of polymer solutions generally fail to describe the early stages of film formation, when hydrodynamic forces control the solution behavior. Using in situ light scattering alongside theoretical and semi-empirical models, it is shown that inertial forces (which initially cause a vertical gradient in the radial solvent velocity within the film) play a significant role in the rate of thinning of the solution. The development of thickness as a function of time of a solute-free liquid (toluene) and a blend of polystyrene and poly(methyl methacrylate) cast from toluene were fitted to different models as a function of toluene partial pressure. In the case of the formation of the polymer blend film, a concentration-dependent (Huggins) viscosity formula was used to account for changes in viscosity during spin coating. A semi-empirical model is introduced, which permits calculation of the solvent evaporation rate and the temporal evolution of the solute volume fraction and solution viscosity.

  8. Effective magnetization damping for a dynamical spin texture in metallic ferromagnet

    NASA Astrophysics Data System (ADS)

    Sukhostavets, Oksana V.; Gonzalez, Julian M.; Guslienko, Konstantin Y.

    2015-10-01

    An additional magnetization damping for an inhomogeneous spin texture in metallic ferromagnets is calculated on the basis of the s-d exchange model. The effect of conduction electrons on the magnetization dynamics is accounted for the case of slowly varying spin texture within adiabatic approximation by using a coordinate transformation to the local quantization axis. The moving magnetic vortex in a circular nanodot made of permalloy is considered as an example. The dependence of the damping on the dot geometrical sizes is obtained. It is found that the additional damping can reach up to 50% of magnitude of the phenomenological Gilbert damping in the Landau-Lifshitz equation of magnetization motion and should be taken into account for any inhomogeneous spin texture dynamics in ferromagnetic metals.

  9. Hole Surface Trapping Dynamics Directly Monitored by Electron Spin Manipulation in CdS Nanocrystals.

    PubMed

    Li, Xiao; Feng, Donghai; Tong, Haifang; Jia, Tianqing; Deng, Li; Sun, Zhenrong; Xu, Zhizhan

    2014-12-18

    A new detection technique, pump-spin orientation-probe ultrafast spectroscopy, is developed to study the hole trapping dynamics in colloidal CdS nanocrystals. The hole surface trapping process spatially separates the electron-hole pairs excited by the pump pulse, leaves the core negatively charged, and thus enhances the electron spin signal generated by the orientation pulse. The spin enhancement transients as a function of the pump-orientation delay reveal a fast and a slow hole trapping process with respective time constants of sub-10 ps and sub-100 ps, orders of magnitude faster than that of carrier recombination. The power dependence of hole trapping dynamics elucidates the saturation process and relative number of traps, and suggests that there are three subpopulations of nanoparticles related to hole surface trapping, one with the fast trapping pathway only, another with the slow trapping pathway only, and the third with both pathways together. PMID:26273979

  10. Numerical study of the dynamics of some long range spin glass models

    NASA Astrophysics Data System (ADS)

    Billoire, Alain

    2015-07-01

    We present results of a Monte Carlo study of the equilibrium dynamics of the one dimensional long-range Ising spin glass model. By tuning a parameter σ , this model interpolates between the mean field Sherrington-Kirkpatrick model and a proxy of the finite dimensional Edward-Anderson model. Activated scaling fits for the behavior of the relaxation time τ as a function of the number of spins N (Namely \\ln (τ )\\propto {{N}\\psi} ) give values of \\psi that are not stable against inclusion of subleading corrections. Critical scaling (τ \\propto {{N}ρ} ) gives more stable fits, at least in the non mean field region. We also present results on the scaling of the time decay of the critical remanent magnetization of the Sherrington-Kirkpatrick model, a case where the simulation can be done with quite large systems and that shows the difficulties in obtaining precise values for dynamical exponents in spin glass models.

  11. Exact quantum dynamics of spin systems using the positive-P representation

    NASA Astrophysics Data System (ADS)

    Ng, Ray; Sorensen, Erik

    2011-03-01

    We discuss a scheme for simulating the exact real time quantum dynamics of interacting quantum spin systems within the positive-P formalism. As model systems we study the transverse field Ising model as well as the Heisenberg model undergoing a quench away from the classical ferromagnetic ordered state. In using the positive-P representation (PPR), the dynamics of the interacting quantum spin system is mapped onto a set of stochastic differential equations (SDEs). The number of which scales linearly with the number of spins, N, compared to an exact solution through diagonalization that in the case of the Heisenberg model would require matrices exponentially large in N. This mapping is exact and can in principle be extended to higher dimensional interacting systems as well as to systems with an explicit coupling to the environment. We compare the results from using a PPR approach based on both the optical coherent states as well as SU(2) Radcliff coherent states.

  12. Probing ultrafast spin dynamics through a magnon resonance in the antiferromagnetic multiferroic HoMnO3

    NASA Astrophysics Data System (ADS)

    Bowlan, P.; Trugman, S. A.; Bowlan, J.; Zhu, J.-X.; Hur, N. J.; Taylor, A. J.; Yarotski, D. A.; Prasankumar, R. P.

    2016-09-01

    We demonstrate an approach for directly tracking antiferromagnetic (AFM) spin dynamics by measuring ultrafast changes in a magnon resonance. We test this idea on the multiferroic HoMnO3 by optically photoexciting electrons, after which changes in the spin order are probed with a THz pulse tuned to a magnon resonance. This reveals a photoinduced change in the magnon line shape that builds up over 5-12 picoseconds, which we show to be the spin-lattice thermalization time, indicating that electrons heat the spins via phonons. We compare our results to previous studies of spin-lattice thermalization in ferromagnetic manganites, giving insight into fundamental differences between the two systems. Our work sheds light on the microscopic mechanism governing spin-phonon interactions in AFMs and demonstrates a powerful approach for directly monitoring ultrafast spin dynamics.

  13. Effects of shielding gas composition on arc profile and molten pool dynamics in gas metal arc welding of steels

    NASA Astrophysics Data System (ADS)

    Wang, L. L.; Lu, F. G.; Wang, H. P.; Murphy, A. B.; Tang, X. H.

    2014-11-01

    In gas metal arc welding, gases of different compositions are used to produce an arc plasma, which heats and melts the workpiece. They also protect the workpiece from the influence of the air during the welding process. This paper models gas metal arc welding (GMAW) processes using an in-house simulation code. It investigates the effects of the gas composition on the temperature distribution in the arc and on the molten pool dynamics in gas metal arc welding of steels. Pure argon, pure CO2 and different mixtures of argon and CO2 are considered in the study. The model is validated by comparing the calculated weld profiles with physical weld measurements. The numerical calculations reveal that gas composition greatly affects the arc temperature profile, heat transfer to the workpiece, and consequently the weld dimension. As the CO2 content in the shielding gas increases, a more constricted arc plasma with higher energy density is generated as a result of the increased current density in the arc centre and increased Lorentz force. The calculation also shows that the heat transferred from the arc to the workpiece increases with increasing CO2 content, resulting in a wider and deeper weld pool and decreased reinforcement height.

  14. Effects of ruthenium seed layer on the microstructure and spin dynamics of thin permalloy films

    SciTech Connect

    Jin Lichuan; Zhang Huaiwu; Tang Xiaoli; Bai Feiming; Zhong Zhiyong

    2013-02-07

    The spin dynamics and microstructure properties of a sputtered 12 nm Ni{sub 81}Fe{sub 19} thin film have been enhanced by the use of a ruthenium seed layer. Both the ferromagnetic resonance field and linewidth are enhanced dramatically as the thickness of ruthenium seed layer is increased. The surface anisotropy energy constant can also be largely tailored from 0.06 to 0.96 erg/cm{sup -2} by changing the seed layer thickness. The changes to the dynamics magnetization properties are caused by both ruthenium seed layer induced changes in the Ni{sub 81}Fe{sub 19} structure properties and surface topography properties. Roughness induced inhomogeneous linewidth broadening is also seen. The damping constant is highly tunable via the ruthenium thickness. This approach can be used to tailor both the structure and spin dynamic properties of thin Ni{sub 81}Fe{sub 19} films over a wide range. And it may benefit the applications of spin dynamics and spin current based devices.

  15. Three-dimensional Computational Fluid Dynamics Investigation of a Spinning Helicopter Slung Load

    NASA Technical Reports Server (NTRS)

    Theorn, J. N.; Duque, E. P. N.; Cicolani, L.; Halsey, R.

    2005-01-01

    After performing steady-state Computational Fluid Dynamics (CFD) calculations using OVERFLOW to validate the CFD method against static wind-tunnel data of a box-shaped cargo container, the same setup was used to investigate unsteady flow with a moving body. Results were compared to flight test data previously collected in which the container is spinning.

  16. Exploring Quantum Many-Body Spin Dynamics with Truncated Wigner Methods

    NASA Astrophysics Data System (ADS)

    Schachenmayer, Johannes

    Recent experiments in atomic, molecular, and optical physics offer controlled and clean environments to experimentally study non-equilibrium dynamics of large many-body quantum spin-models with variable range interactions. Thus, efficient computation of such dynamics is of great importance. While in one dimension, time-dependent density matrix renormalization group methods (t-DMRG) have proven effective under certain conditions, computing dynamics in higher dimensional systems remains an outstanding challenge. Recently we formulated the discrete truncated Wigner approximation (DTWA), a semiclassical method based on the truncated Wigner approximation (TWA) that has been proven to be surprisingly accurate in predicting quench dynamics in high-dimensional lattices with up to tens of thousands of quantum spins. Here, we introduce the DTWA and show how it can compute time-evolution of quantum states in experiments that engineer spin-models with polar molecules in optical lattices or with ions in two-dimensional Penning traps. We show, how the DTWA can provide results for the time-evolution of classical and quantum correlations in quench experiments in regimes where other numerical methods are generally unreliable. We report on progress of how to incorporate higher order corrections to the method, and how to adapt it to systems with both spin and bosonic degrees of freedom.

  17. REACTOR SHIELD

    DOEpatents

    Wigner, E.P.; Ohlinger, L.E.; Young, G.J.; Weinberg, A.M.

    1959-02-17

    Radiation shield construction is described for a nuclear reactor. The shield is comprised of a plurality of steel plates arranged in parallel spaced relationship within a peripheral shell. Reactor coolant inlet tubes extend at right angles through the plates and baffles are arranged between the plates at right angles thereto and extend between the tubes to create a series of zigzag channels between the plates for the circulation of coolant fluid through the shield. The shield may be divided into two main sections; an inner section adjacent the reactor container and an outer section spaced therefrom. Coolant through the first section may be circulated at a faster rate than coolant circulated through the outer section since the area closest to the reactor container is at a higher temperature and is more radioactive. The two sections may have separate cooling systems to prevent the coolant in the outer section from mixing with the more contaminated coolant in the inner section.

  18. Magnetic-field-induced dynamical instabilities in an antiferromagnetic spin-1 Bose-Einstein condensate

    NASA Astrophysics Data System (ADS)

    Pu, Zhengguo; Zhang, Jun; Yi, Su; Wang, Dajun; Zhang, Wenxian

    2016-05-01

    We theoretically investigate four types of dynamical instability, in particular the periodic and oscillatory type IO, in an antiferromagnetic spin-1 Bose-Einstein condensate in a nonzero magnetic field, by employing the coupled-mode theory and numerical method. This is in sharp contrast to the dynamical stability of the same system in zero field. Remarkably, a pattern transition from a periodic dynamical instability IO to a uniform one IIIO occurs at a critical magnetic field. All four types of dynamical instability and the pattern transition are ready to be detected in 23Na condensates within the availability of the current experimental techniques.

  19. Spin-system dynamics and fault detection in threshold networks

    SciTech Connect

    Kirkland, Steve; Severini, Simone

    2011-01-15

    We consider an agent on a fixed but arbitrary node of a known threshold network, with the task of detecting an unknown missing link. We obtain analytic formulas for the probability of success when the agent's tool is the free evolution of a single excitation on an XX spin system paired with the network. We completely characterize the parameters, which allows us to obtain an advantageous solution. From the results emerges an optimal (deterministic) algorithm for quantum search, from which a quadratic speedup with respect to the optimal classical analog and in line with well-known results in quantum computation is gained. When attempting to detect a faulty node, the chosen setting appears to be very fragile and the probability of success too small to be of any direct use.

  20. Energy dynamics in the Heisenberg-Kitaev spin chain

    NASA Astrophysics Data System (ADS)

    Steinigeweg, Robin; Brenig, Wolfram

    2016-06-01

    We study the Heisenberg-Kitaev spin chain in order to uncover the interplay between two qualitatively different integrable points in the physics of heat transport in one dimension. Focusing on high temperatures and using analytical as well as numerical approaches within linear response theory, we explore several directions in parameter space including exchange-coupling ratios, anisotropies, and external magnetic fields. We show the emergence of purely ballistic energy transport at all integrable points, manifest in pronounced Drude weights and low-frequency suppression of regular-conductivity contributions. Moreover, off integrability, we find extended quantum chaotic regions with vanishing Drude weights and well-defined dc conductivities. In the vicinity of the Kitaev point, we observe clear signatures of the topological gap in the response function. This gap coexists with a nonzero Drude weight in the Kitaev chain.

  1. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    DOE PAGESBeta

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-24

    In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal controlmore » scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.« less

  2. Dynamic strain-mediated coupling of a single diamond spin to a mechanical resonator

    PubMed Central

    Ovartchaiyapong, Preeti; Lee, Kenneth W.; Myers, Bryan A.; Jayich, Ania C. Bleszynski

    2014-01-01

    The development of hybrid quantum systems is central to the advancement of emerging quantum technologies, including quantum information science and quantum-assisted sensing. The recent demonstration of high-quality single-crystal diamond resonators has led to significant interest in a hybrid system consisting of nitrogen–vacancy centre spins that interact with the resonant phonon modes of a macroscopic mechanical resonator through crystal strain. However, the nitrogen–vacancy spin–strain interaction has not been well characterized. Here, we demonstrate dynamic, strain-mediated coupling of the mechanical motion of a diamond cantilever to the spin of an embedded nitrogen–vacancy centre. Via quantum control of the spin, we quantitatively characterize the axial and transverse strain sensitivities of the nitrogen–vacancy ground-state spin. The nitrogen–vacancy centre is an atomic scale sensor and we demonstrate spin-based strain imaging with a strain sensitivity of 3 × 10−6 strain Hz−1/2. Finally, we show how this spin-resonator system could enable coherent spin–phonon interactions in the quantum regime. PMID:25034828

  3. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    SciTech Connect

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-24

    In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.

  4. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    NASA Astrophysics Data System (ADS)

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-01

    We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ˜0.7 ms up to ˜30 ms . We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.

  5. Resolving the role of femtosecond heated electrons in ultrafast spin dynamics

    PubMed Central

    Mendil, J.; Nieves, P.; Chubykalo-Fesenko, O.; Walowski, J.; Santos, T.; Pisana, S.; Münzenberg, M.

    2014-01-01

    Magnetization manipulation is essential for basic research and applications. A fundamental question is, how fast can the magnetization be reversed in nanoscale magnetic storage media. When subject to an ultrafast laser pulse, the speed of the magnetization dynamics depends on the nature of the energy transfer pathway. The order of the spin system can be effectively influenced through spin-flip processes mediated by hot electrons. It has been predicted that as electrons drive spins into the regime close to almost total demagnetization, characterized by a loss of ferromagnetic correlations near criticality, a second slower demagnetization process takes place after the initial fast drop of magnetization. By studying FePt, we unravel the fundamental role of the electronic structure. As the ferromagnet Fe becomes more noble in the FePt compound, the electronic structure is changed and the density of states around the Fermi level is reduced, thereby driving the spin correlations into the limit of critical fluctuations. We demonstrate the impact of the electrons and the ferromagnetic interactions, which allows a general insight into the mechanisms of spin dynamics when the ferromagnetic state is highly excited, and identifies possible recording speed limits in heat-assisted magnetization reversal. PMID:24496221

  6. Advances and applications of dynamic-angle spinning nuclear magnetic resonance

    SciTech Connect

    Baltisberger, J.H.

    1993-06-01

    This dissertation describes nuclear magnetic resonance experiments and theory which have been developed to study quadrupolar nuclei (those nuclei with spin greater than one-half) in the solid state. Primarily, the technique of dynamic-angle spinning (DAS) is extensively reviewed and expanded upon in this thesis. Specifically, the improvement in both the resolution (two-dimensional pure-absorptive phase methods and DAS angle choice) and sensitivity (pulse-sequence development), along with effective spinning speed enhancement (again through choice of DAS conditions or alternative multiple pulse schemes) of dynamic-angle spinning experiment was realized with both theory and experimental examples. The application of DAS to new types of nuclei (specifically the {sup 87}Rb and {sup 85}Rb nuclear spins) and materials (specifically amorphous solids) has also greatly expanded the possibilities of the use of DAS to study a larger range of materials. This dissertation is meant to demonstrate both recent advances and applications of the DAS technique, and by no means represents a comprehensive study of any particular chemical problem.

  7. Spin-Orbit Interactions and Quantum Spin Dynamics in Cold Ion-Atom Collisions

    NASA Astrophysics Data System (ADS)

    Tscherbul, Timur V.; Brumer, Paul; Buchachenko, Alexei A.

    2016-09-01

    We present accurate ab initio and quantum scattering calculations on a prototypical hybrid ion-atom system Yb+ -Rb, recently suggested as a promising candidate for the experimental study of open quantum systems, quantum information processing, and quantum simulation. We identify the second-order spin-orbit (SO) interaction as the dominant source of hyperfine relaxation in cold Yb+ -Rb collisions. Our results are in good agreement with recent experimental observations [L. Ratschbacher et al., Phys. Rev. Lett. 110, 160402 (2013)] of hyperfine relaxation rates of trapped Yb+ immersed in an ultracold Rb gas. The calculated rates are 4 times smaller than is predicted by the Langevin capture theory and display a weak T-0.3 temperature dependence, indicating significant deviations from statistical behavior. Our analysis underscores the deleterious nature of the SO interaction and implies that light ion-atom combinations such as Yb+ -Li should be used to minimize hyperfine relaxation and decoherence of trapped ions in ultracold atomic gases.

  8. Quantum spin dynamics at terahertz frequencies in 2D hole gases and improper ferroelectrics

    NASA Astrophysics Data System (ADS)

    Lloyd-Hughes, J.

    2015-08-01

    Terahertz time-domain spectroscopy permits the excitations of novel materials to be examined with exquisite precision. Improper ferroelectric materials such as cupric oxide (CuO) exhibit complex magnetic ground states. CuO is antiferromagnetic below 213K, but has an incommensurate cycloidal magnetic phase between 213K and 230K. Remarkably, the cycloidal magnetic phase drives ferroelectricity, where the material becomes polar. Such improper multiferroics are of great contemporary interest, as a better understanding of the science of magnetoelectric materials may lead to their application in actuators, sensors and solid state memories. Improper multiferroics also have novel quasiparticle excitations: electromagnons form when spin-waves become electric-dipole active. By examining the dynamic response of spins as they interact with THz radiation we gain insights into the underlying physics of multi-ferroics. In contrast to improper ferroelectrics, where magnetism drives structural inversion asymmetry (SIA), two-dimensional electronic systems can exhibit non-degenerate spin states as a consequence of SIA created by strain and/or electric fields. We identify and explore the influence of the Rashba spin-orbit interaction upon cyclotron resonance at terahertz frequencies in high-mobility 2D hole gases in germanium quantum wells. An enhanced Rashba spin-orbit interaction can be linked to the strain of the quantum well, while a time-frequency decomposition method permitted the dynamical formation and decay of spin-split cyclotron resonances to be tracked on picosecond timescales. Long spin-decoherence times concurrent with high hole mobilities highlight the potential of Ge quantum wells in spintronics.

  9. First principles study of atomic-scale nanowires and dynamical transverse spin susceptibility

    NASA Astrophysics Data System (ADS)

    Ke, Liqin

    This dissertation includes two independent theoretical studies: (a) structure and electron transport in Au and Co nanowires by using the local-density approximation (LDA), and (b) studies of the dynamical transverse spin susceptibility in Fe, Ni, Co and FeSe. Ballistic conductance calculations of infinite zigzag chains of Co and Au, and multi-atom Au nanowires, were calculated within the Landauer-Buttiker formalism. The Co chain was spin polarized, and the majority spin channel exhibits quantized conductance. But because of the close spacing of Co d levels, the minority channel does not. In contrast, Au is not spin polarized, and shows well-behaved quantization. The deformation of an atomic Au wire placed between Au electrodes was investigated theoretically. It was found that the lowest phonon eigenstates are associated with lateral motion of atoms in the middle of the chain. Large displacements which resulted in wire breakage were studied, and the energy barrier associated with this process has been calculated. At certain stages of the wire breaking process, atomic fluctuations become very large, which results in an intrinsic conductance fluctuation, even at arbitrarily low temperature. The theoretical background and calculational formalism of the dynamical transverse spin susceptibility is presented in two approximations, the Rigid Spin Approximation (RSA) and the time-dependent LDA. The latter was implemented with a recently developed full product basis (FPB) method. In the RSA case, the exchange-correlation kernel is determined indirectly from a sum rule. The theory was applied to bcc-Fe, fcc-Ni, hcp-Co, and to FeSe in the Neel magnetic structure. In the FeSe case, intra-pocket and inter-pocket mechanisms were found to govern the low energy bare susceptibility. The enhanced susceptibility was found to consist of some admixture of Stoner excitations and spin wave parts.

  10. Dynamics of intramolecular spin exchange interaction of a nitronyl nitroxide diradical in solution and on surfaces.

    PubMed

    Lloveras, V; Badetti, E; Veciana, J; Vidal-Gancedo, J

    2016-03-01

    In this paper we report the study of the dynamics of a thermally modulated intramolecular spin exchange interaction of a novel diradical nitronyl nitroxide-substituted disulfide in solution and when it is grafted on a gold surface. The structure of this diradical was designed to have flexible chains leading to intramolecular collisions and hence spin exchange interaction, and with an appropriate binding group to be grafted on the gold surface to study its behavior on the surface. In solution, this diradical shows a strong spin exchange interaction between both radicals which is modulated by temperature, but also gold nanoparticles (AuNPs) functionalized with this diradical permit investigation of such a phenomenon in surface-grafted radicals. The spin-labelled AuNP synthesis was optimized to obtain high coverage of spin labels to lead to high spin exchange interaction. The obtained AuNPs were studied by Electron Paramagnetic Resonance (EPR), UV-Vis, and IR spectroscopies, HR-TEM microscopy, Cyclic Voltammetry (CV), Energy Dispersive X-ray analysis (EDX) and Thermogravimetric Analysis (TGA). This inorganic-organic hybrid material also showed dipolar interactions between its radicals which were confirmed by the appearance in the EPR spectra of an |Δms| = 2 transition at half-field. This signal gives direct evidence of the presence of a high-spin state and permitted us to study the nature of the magnetic coupling between the spins which was found to be antiferromagnetic. Self-Assembled Monolayers (SAMs) of these radicals on the Au (111) substrate were also prepared and studied by contact angle, X-Ray Photoelectron Spectroscopy (XPS), Time-of-Flight Secondary Ion Mass Spectrometry (ToF-SIMS), Cyclic Voltammetry and EPR. The magnetic as well as the electrochemical properties of the hybrid surfaces were studied and compared with the properties of this diradical in solution. Analogies between the properties of AuNPs with high coverage of radicals and those of SAM were

  11. Static and dynamic properties of interacting spin-1 bosons in an optical lattice

    NASA Astrophysics Data System (ADS)

    Natu, Stefan S.; Pixley, J. H.; Das Sarma, S.

    2015-04-01

    We study the physics of interacting spin-1 bosons in an optical lattice using a variational Gutzwiller technique. We compute the mean-field ground state wave function and discuss the evolution of the condensate, spin, nematic, and singlet order parameters across the superfluid-Mott transition. We then extend the Gutzwiller method to derive the equations governing the dynamics of low energy excitations in the lattice. Linearizing these equations, we compute the excitation spectra in the superfluid and Mott phases for both ferromagnetic and antiferromagnetic spin-spin interactions. In the superfluid phase, we recover the known excitation spectrum obtained from Bogoliubov theory. In the nematic Mott phase, we obtain gapped, quadratically dispersing particle and hole-like collective modes, whereas in the singlet Mott phase, we obtain a nondispersive gapped mode, corresponding to the breaking of a singlet pair. For the ferromagnetic Mott insulator, the Gutzwiller mean-field theory only yields particle-hole-like modes but no Goldstone mode associated with long-range spin order. To overcome this limitation, we supplement the Gutzwiller theory with a Schwinger boson mean-field theory which captures superexchange-driven fluctuations. In addition to the gapped particle-hole-like modes, we obtain a gapless quadratically dispersing ferromagnetic spin-wave Goldstone mode. We discuss the evolution of the singlet gap, particle-hole gap, and the effective mass of the ferromagnetic Goldstone mode as the superfluid-Mott phase boundary is approached from the insulating side. We discuss the relevance and validity of Gutzwiller mean-field theories to spinful systems, and potential extensions of this framework to include more exotic physics which appears in the presence of spin-orbit coupling or artificial gauge fields.

  12. Cooperative dynamics in polymer melts: a comparison of theoretical predictions with Neutron Spin Echo experiments

    NASA Astrophysics Data System (ADS)

    Guenza, Marina

    2009-03-01

    We present a comparison between theoretical predictions of the Generalized Langevin Equation for Cooperative Dynamics (CDGLE) and Neutron Spin Echo data of dynamics structure factors for polyethylene melts. Experiments, peformed by Zamponi end coowrkers, cover an extended range of length- and time-scales providing a compelling test for the theoretical approach. Samples investigated include chains with increasing molecular weights, undergoing dynamics across the unentangled to entangled transition. Measured center-of- mass mean-square displacements display a crossover from subdiffusive to diffusive dynamics. The Generalized Langevin Equation for Cooperative Dynamics relates this anomalous diffusion to the presence of the interpolymer potential, which correlates the dynamics of a group of slowly diffusing molecules in a dynamically heterogeneous liquid. Theoretical predictions of the subdiffusive behavior, its crossover to free diffusion, and of the number of macromolecules undergoing cooperative motion are in quantitative agreement with experiments.

  13. Continuum description of ionic and dielectric shielding for molecular-dynamics simulations of proteins in solution.

    PubMed

    Egwolf, Bernhard; Tavan, Paul

    2004-01-22

    We extend our continuum description of solvent dielectrics in molecular-dynamics (MD) simulations, which has provided an efficient and accurate solution of the Poisson equation, to ionic solvents as described by the linearized Poisson-Boltzmann (LPB) equation. We start with the formulation of a general theory for the electrostatics of an arbitrarily shaped molecular system, which consists of partially charged atoms and is embedded in a LPB continuum. This theory represents the reaction field induced by the continuum in terms of charge and dipole densities localized within the molecular system. Because these densities cannot be calculated analytically for systems of arbitrary shape, we introduce an atom-based discretization and a set of carefully designed approximations. This allows us to represent the densities by charges and dipoles located at the atoms. Coupled systems of linear equations determine these multipoles and can be rapidly solved by iteration during a MD simulation. The multipoles yield the reaction field forces and energies. Finally, we scrutinize the quality of our approach by comparisons with an analytical solution restricted to perfectly spherical systems and with results of a finite difference method.

  14. Neutron spin echo study of the dynamics of undercooled selenium

    NASA Astrophysics Data System (ADS)

    Simon, Ch.; Faivre, G.; Zorn, R.; Batallan, F.; Legrand, J. F.

    1992-03-01

    We present neutron spin echo measurements on the structural relaxation of undercooled liquid selenium above glass transition. We find a two-stage relaxation process essentially similar to that generally observed in liquids, except for the fact that the slow-stage characteristic time tau_1 varies with the temperature T more slowly than η(T)/T, where η(T) is the macroscopic viscosity. We interpret this apparent discrepancy with respect to the usually found scaling law as the manifestation of the equilibrium-polymer nature of liquid selenium. On the other hand, the data suggest that the Kohlrausch exponent of the slow stage is temperature dependent. Concerning the rapid stage of the relaxation, we show that a possible alternative to the mode-coupling interpretation is to attribute it to the existence of local inhomogeneities of the density close to the glass transition. Nous présentons des résultats de mesures au spectromètre à écho de spin sur la relaxation structurale du sélenium en surfusion près de la transition vitreuse. Nous trouvons une relaxation en deux étapes, essentiellement conforme à celle trouvée antérieurement dans d'autres liquides, à ceci près que le temps caractéristique tau_1 du stade lent varie avec la température T plus lentement que η(T)/T, où η(T) est la viscosité macroscopique. Nous interprétons cet écart apparent à la loi d'échelle généralement observée comme la manifestation du fait que le sélénium liquide est un polymère d'équilibre. L'analyse des données suggège d'autre part que l'exposant de Kohlrausch du stade lent dépend de la température. Quant au stade rapide de la relaxation, nous montrons qu'il peut être interprété, sans recourir à la théorie du couplage de modes, par l'existance d'hétérogénéités locales de la densité au voisinage de la transition vitreuse.

  15. Backbone Dynamics of Alamethicin Bound to Lipid Membranes: Spin-Echo Electron Paramagnetic Resonance of TOAC-Spin Labels

    PubMed Central

    Bartucci, Rosa; Guzzi, Rita; De Zotti, Marta; Toniolo, Claudio; Sportelli, Luigi; Marsh, Derek

    2008-01-01

    Alamethicin F50/5 is a hydrophobic peptide that is devoid of charged residues and that induces voltage-dependent ion channels in lipid membranes. The peptide backbone is likely to be involved in the ion conduction pathway. Electron spin-echo spectroscopy of alamethicin F50/5 analogs in which a selected Aib residue (at position n = 1, 8, or 16) is replaced by the TOAC amino-acid spin label was used to study torsional dynamics of the peptide backbone in association with phosphatidylcholine bilayer membranes. Rapid librational motions of limited angular amplitude were observed at each of the three TOAC sites by recording echo-detected spectra as a function of echo delay time, 2τ. Simulation of the time-resolved spectra, combined with conventional EPR measurements of the librational amplitude, shows that torsional fluctuations of the peptide backbone take place on the subnanosecond to nanosecond timescale, with little temperature dependence. Associated fluctuations in polar fields from the peptide could facilitate ion permeation. PMID:18096632

  16. Dynamical properties of three terminal magnetic tunnel junctions: Spintronics meets spin-orbitronics

    SciTech Connect

    Tomasello, R.; Carpentieri, M.; Finocchio, G.

    2013-12-16

    This Letter introduces a micromagnetic model able to characterize the magnetization dynamics in three terminal magnetic tunnel junctions, where the effects of spin-transfer torque and spin-orbit torque are taken into account. Our results predict that the possibility to separate electrically those two torque sources is very promising from a technological point of view for both next generation of nanoscale spintronic oscillators and microwave detectors. A scalable synchronization scheme based on the parallel connection of those three terminal devices is also proposed.

  17. Reprint of : Transient dynamics of spin-polarized injection in helical Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Calzona, A.; Carrega, M.; Dolcetto, G.; Sassetti, M.

    2016-08-01

    We analyze the time evolution of spin-polarized electron wave packets injected into the edge states of a two-dimensional topological insulator. In the presence of electron interactions, the system is described as a helical Luttinger liquid and injected electrons fractionalize. However, because of the presence of metallic detectors, no evidences of fractionalization are encoded in dc measurements, and in this regime the system does not show deviations from its non-interacting behavior. Nevertheless, we show that the helical Luttinger liquid nature emerges in the transient dynamics, where signatures of charge/spin fractionalization can be clearly identified.

  18. Spin-Dependent Studies of the Dynamics of He+ Ion Neutralization at Surfaces

    NASA Astrophysics Data System (ADS)

    Lancaster, J. C.; Kontur, F. J.; Nordlander, P.; Walters, G. K.; Dunning, F. B.

    2001-05-01

    Spin-labelling techniques, specifically the use of electron-spin-polarized ^4He^+ ions coupled with energy-resolved measurements of the ejected electron polarization, are used to study the dynamics of He^+ neutralization at surfaces. The He^+ ions are produced by Penning ionization in collisions between polarized He(2^3S) metastable atoms contained in a weak rf-excited discharge. Studies of Cu(100), Au(100), Al(100) and sub-monolayer alkali-covered Al(100) surfaces are underway to investigate the role of surface electronic structure, work function and adsorbate coverage in determining the neutralization dynamics. The data for clean surfaces display the same general behavior and reveal a marked correlation in the spins of the electrons involved in Auger neutralization of the He^+ ions. A pronounced energy dependence in the ejected electron polarization also is observed. These results are explained by model calculations which show the presence of the (polarized) He^+ ion leads to strong, spin-dependent perturbations in the local surface electronic structure. Quite different behavior is observed at alkali-covered surfaces, and further work is underway to identify the underlying dynamics.

  19. Noise in optical quantum memories based on dynamical decoupling of spin states

    NASA Astrophysics Data System (ADS)

    Zambrini Cruzeiro, Emmanuel; Fröwis, Florian; Timoney, Nuala; Afzelius, Mikael

    2016-11-01

    Long-lived optical quantum memories are of great importance for scalable distribution of entanglement over remote networks (e.g. quantum repeaters). Long-lived storage generally relies on storing the optical states as spin excitations since these often exhibit long coherence times. To extend the storage time beyond the intrinsic spin dephasing time one can use dynamical decoupling techniques. However, it has been shown that dynamical decoupling introduces noise in optical quantum memories based on ensembles of atoms. In this article, a simple model is proposed to calculate the resulting signal-to-noise ratio, based on intrinsic quantum memory parameters such as the optical depth of the ensemble. We also characterize several dynamical decoupling sequences that are efficient in reducing this particular noise. Our calculations indicate that it should be feasible to reach storage times well beyond one second under reasonable experimental conditions.

  20. Deployment dynamics of a simplified spinning IKAROS solar sail via absolute coordinate based method

    NASA Astrophysics Data System (ADS)

    Zhao, Jiang; Tian, Qiang; Hu, Hai-Yan

    2013-02-01

    The spinning solar sail of large scale has been well developed in recent years. Such a solar sail can be considered as a rigid-flexible multibody system mainly composed of a spinning central rigid hub, a number of flexible thin tethers, sail membranes, and tip masses. A simplified interplanetary kite-craft accelerated by radiation of the Sun (IKAROS) model is established in this study by using the absolute-coordinate-based (ACB) method that combines the natural coordinate formulation (NCF) describing the central rigid hub and the absolute nodal coordinate formulation (ANCF) describing flexible parts. The initial configuration of the system in the second-stage deployment is determined through both dynamic and static analyses. The huge set of stiff equations of system dynamics is solved by using the generalized-alpha method, and thus the deployment dynamics of the system can be well understood.

  1. Simulation of spin dynamics: a tool in MRI system development

    NASA Astrophysics Data System (ADS)

    Stöcker, Tony; Vahedipour, Kaveh; Shah, N. Jon

    2011-05-01

    Magnetic Resonance Imaging (MRI) is a routine diagnostic tool in the clinics and the method of choice in soft-tissue contrast medical imaging. It is an important tool in neuroscience to investigate structure and function of the living brain on a systemic level. The latter is one of the driving forces to further develop MRI technology, as neuroscience especially demands higher spatiotemporal resolution which is to be achieved through increasing the static main magnetic field, B0. Although standard MRI is a mature technology, ultra high field (UHF) systems, at B0 >= 7 T, offer space for new technical inventions as the physical conditions dramatically change. This work shows that the development strongly benefits from computer simulations of the measurement process on the basis of a semi-classical, nuclear spin-1/2 treatment given by the Bloch equations. Possible applications of such simulations are outlined, suggesting new solutions to the UHF-specific inhomogeneity problems of the static main field as well as the high-frequency transmit field.

  2. A Conservative Solution to the Stochastic Dynamical Reduction Problem. Case of Spin- z Measurement of a Spin-1/2 Particle

    NASA Astrophysics Data System (ADS)

    Halabi, T.

    2013-10-01

    Stochastic dynamical reduction for the case of spin- z measurement of a spin-1/2 particle describes a random walk on the spin- z axis. The measurement’s result depends on which of the two points: spin- z=± ħ/2 is reached first. Born’s rule is recovered as long as the expected step size in spin- z is independent of proximity to endpoints. Here, we address the questions raised by this description: (1) When is collapse triggered, and what triggers it? (2) Why is the expected step size in spin- z (as opposed to polar angle) independent of proximity to endpoints? (3) Why does spin “lock” in the vertical directions? The difficulties associated with (1) are rooted, as is Bell’s theorem, in the time-asymmetric assumption that the present distribution over hidden variables is independent of future settings. We believe, a priori of any of the experiments of modern physics, that such a time-asymmetric assumption is dubious when probing the microscopic scale. As for (2) and (3), they are simultaneously resolved by abandoning the fundamental distinction drawn between spin and spatial angular momentum, and by appealing to very tiny (in both magnitude and spatial extent) but numerous patches of magnetic noise in the Stern-Gerlach’s field.

  3. Effects of stereoelectronic interactions on the relativistic spin-orbit and paramagnetic components of the (13)C NMR shielding tensors of dihaloethenes.

    PubMed

    Viesser, Renan V; Ducati, Lucas C; Autschbach, Jochen; Tormena, Cláudio F

    2015-07-15

    In this study, stereoelectronic interactions were considered to explain the experimental difference in the magnitude of the known heavy-atom effect on the (13)C NMR chemical shifts in cis- and trans-1,2-dihaloethene isomers (halo = F, Cl, Br or I). The experimental values were compared to the calculated values with various DFT functionals using both the nonrelativistic approach (NR) and the relativistic approximations SR-ZORA (SR) and SO-ZORA (SO). NBO and NLMO contributions to the (13)C NMR shielding tensors were determined to assess which stereoelectronic interactions have a more important effect on the shielding tensor in each principal axis system (PAS) coordinate. These analyses associated with the orbital rotation model and the HOMO-LUMO energy gap enable rationalization of trends between cis and trans isomers from fluorine to iodine derivatives. Both paramagnetic and SO shielding terms were responsible for the observed trends. It was possible to conclude that the steric interactions between the two iodine atoms and the hyperconjugative interactions involving the halogen lone pairs (LP(X)) and πC[double bond, length as m-dash]C*, σC[double bond, length as m-dash]C* and σC-X* antibonding orbitals are responsible for the lower (13)C NMR shielding for the cis isomers of the bromine and the iodine compounds than that of the trans isomers.

  4. Overall and internal dynamics of DNA as monitored by five-atom-tethered spin labels.

    PubMed Central

    Keyes, R S; Bobst, E V; Cao, Y Y; Bobst, A M

    1997-01-01

    Electron paramagnetic resonance (EPR) spectra of the two-atom-tethered six-membered ring thymidylate spin label (DUMTA) incorporated into duplexes of different sizes were found to display a helix length dependence and a local-order parameter S = 0.32 +/- 0.01 for B-DNA based on the dynamic cylinder model (Keyes, R. S., and A. M. Bobst. 1995. Detection of internal and overall dynamics of a two-atom-tethered spin-labeled DNA. Biochemistry. 34:9265-9276). This sensitivity to size, which reflects global tumbling, is now reported for the more flexible five-atom-tethered five-membered ring thymidylate spin label (DUAP) that can be readily incorporated enzymatically and sequence specifically into nucleic acids of different sizes. The DUAPs containing B-DNA systems were simulated with the same dynamic cylinder model, giving S = 0.20 +/- 0.01 for the more flexibly tethered spin label. This shows that S is dependent on tether length but not on global motion. An analysis with the same motional model of the B-Z transition in a (dG-dC)n polymer containing the five-atom-tethered six-membered ring cytidylate spin label (DCAT) (Strobel, O. K., R. S. Keyes, and A. M. Bobst. 1990b. Base dynamics of local Z-DNA conformations as detected by electron paramagnetic resonance with spin-labeled deoxycytidine analogues. Biochemistry. 29:8522-8528) revealed an increase in S from 0.15 +/- 0.01 to 0.26 +/- 0.01 in response to the B- to Z-DNA transition. This indicates that S is not only sensitive to tether length, but also to conformational changes in DNA. Both the DUAP- and the DCAT-labeled systems were also simulated with a base disk model. From the DUAP spectral series, the perpendicular component of the correlation time tau perpendicular describing the spin-labeled base diffusion was found to be sensitive to global tumbling, confirming earlier results obtained with DUMTA. The DCAT polymer results demonstrated that tau perpendicular monitors a conformational change from B- to Z

  5. What can we learn about the dynamics of transported spins by measuring shot noise in spin-orbit-coupled nanostructures?

    NASA Astrophysics Data System (ADS)

    Nikolić, Branislav K.; Dragomirova, Ralitsa L.

    2009-06-01

    We review recent studies of the shot noise of spin-polarized charge currents and pure spin currents in multiterminal semiconductor nanostructures, while focusing on the effects brought by the intrinsic Rashba spin-orbit (SO) coupling and/or extrinsic SO scattering off impurities in two-dimensional electron gas (2DEG) based devices. By generalizing the scattering theory of quantum shot noise to include the full spin-density matrix of electrons injected from a spin-filtering electrode, we show how decoherence and dephasing in the course of spin precession can lead to the substantial enhancement of the Fano factor (noise-to-current ratio) of spin-polarized charge currents. These processes are suppressed by decreasing the width of the diffusive Rashba wire, so that purely electrical measurement of the shot noise in a ferromagnet|SO-coupled-diffusive-wire|paramagnet setup can quantify the degree of quantum coherence of transported spin through a remarkable one-to-one correspondence between the purity of the spin state and the Fano factor. In four-terminal SO-coupled nanostructures, injection of unpolarized charge current through the longitudinal leads is responsible not only for the pure spin Hall current in the transverse leads, but also for nonequilibrium random time-dependent current fluctuations. The analysis of the shot noise of transverse pure spin Hall current and zero charge current, or transverse spin current and non-zero charge Hall current, driven by unpolarized or spin-polarized injected longitudinal charge current, respectively, reveals a unique experimental tool to differentiate between the intrinsic Rashba and extrinsic SO mechanisms underlying the spin Hall effect in 2DEG devices. When the intrinsic mechanisms responsible for spin precession start to dominate the spin Hall effect, they also enhance the shot noise of transverse spin and charge transport in multiterminal geometries. Finally, we discuss the shot noise of transverse spin and zero charge

  6. Using synthetic model systems to understand charge separation and spin dynamics in photosynthetic reaction centers.

    SciTech Connect

    Wasielewski, M. R.

    1998-08-27

    Our current work in modeling reaction center dynamics has resulted in the observation of each major spin-dependent photochemical pathway that is observed in reaction centers. The development of new, simpler model systems has permitted us to probe deeply into the mechanistic issues that drive these dynamics. Based on these results we have returned to biomimetic chlorophyll-based electron donors to mimic these dynamics. Future studies will focus on the details of electronic structure and energetic of both the donor-acceptor molecules and their surrounding environment that dictate the mechanistic pathways and result in efficient photosynthetic charge separation.

  7. Quantum spin dynamics and entanglement generation with hundreds of trapped ions.

    PubMed

    Bohnet, Justin G; Sawyer, Brian C; Britton, Joseph W; Wall, Michael L; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J

    2016-06-10

    Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of (9)Be(+) ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods.

  8. Short-time spin dynamics in strongly correlated few-fermion systems.

    PubMed

    Peotta, Sebastiano; Rossini, Davide; Silvi, Pietro; Vignale, G; Fazio, Rosario; Polini, Marco

    2012-06-15

    The nonequilibrium spin dynamics of a one-dimensional system of repulsively interacting fermions is studied by means of density-matrix renormalization group simulations. We focus on the short-time decay of the oscillation amplitudes of the centers of mass of spin-up and spin-down fermions. Because of many body effects, the decay is found to evolve from quadratic to linear in time, and eventually back to quadratic as the strength of the interaction increases. The characteristic rate of the decay increases linearly with the strength of repulsion in the weak-coupling regime, while it is inversely proportional to it in the strong-coupling regime. Our predictions can be tested in experiments on tunable ultracold few-fermion systems in one-dimensional traps. PMID:23004286

  9. Quantum spin dynamics and entanglement generation with hundreds of trapped ions

    NASA Astrophysics Data System (ADS)

    Bohnet, Justin G.; Sawyer, Brian C.; Britton, Joseph W.; Wall, Michael L.; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J.

    2016-06-01

    Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of 9Be+ ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods.

  10. Saturation Recovery EPR and Nitroxide Spin Labeling for Exploring Structure and Dynamics in Proteins.

    PubMed

    Yang, Zhongyu; Bridges, Michael; Lerch, Michael T; Altenbach, Christian; Hubbell, Wayne L

    2015-01-01

    Experimental techniques capable of determining the structure and dynamics of proteins are continuously being developed in order to understand protein function. Among existing methods, site-directed spin labeling in combination with saturation recovery (SR) electron paramagnetic resonance spectroscopy contributes uniquely to the determination of secondary and tertiary protein structure under physiological conditions, independent of molecular weight and complexity. In addition, SR of spin labeled proteins was recently demonstrated to be sensitive to conformational exchange events with characteristic lifetimes on the order of μs, a time domain that presents a significant challenge to other spectroscopic techniques. In this chapter, we present the theoretical background necessary to understand the capabilities of SR as applied to spin labeled proteins, the instrumental requirements, and practical experimental considerations necessary to obtain interpretable data, and the use of SR to obtain information on protein: (1) secondary structure via solvent accessibility measurements, (2) tertiary structure using interspin distance measurements, and (3) conformational exchange. PMID:26477246

  11. Quantum spin dynamics and entanglement generation with hundreds of trapped ions.

    PubMed

    Bohnet, Justin G; Sawyer, Brian C; Britton, Joseph W; Wall, Michael L; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J

    2016-06-10

    Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of (9)Be(+) ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods. PMID:27284189

  12. Anomalously slow spin dynamics and short-range correlations in the quantum spin ice systems Yb2Ti2O7 and Yb2Sn2O7

    NASA Astrophysics Data System (ADS)

    Maisuradze, A.; Dalmas de Réotier, P.; Yaouanc, A.; Forget, A.; Baines, C.; King, P. J. C.

    2015-09-01

    We report a positive muon spin relaxation and rotation (μ SR ) study of the quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field response. In agreement with earlier reports, data recorded in small longitudinal fields evidence anomalously slow spin dynamics in the microsecond range below the temperature Tc at which the specific heat displays an intense peak, namely Tc=0.24 K and 0.15 K, respectively, for the two systems. We found that slow dynamics extends above Tc up to at least 0.7 K for both compounds. The conventional dynamical Gaussian Kubo-Toyabe model describes the μ SR spectra recorded above Tc. At lower temperatures a published analytical extension of the Gaussian Kubo-Toyabe model provides a good description, consistent with the existence of short-range magnetic correlations. While the physical response of the two systems is qualitatively the same, Yb2Ti2O7 exhibits a much larger local magnetic susceptibility than Yb2Sn2O7 below Tc. Considering previously reported ac susceptibility, neutron scattering, and μ SR results, we suggest the existence of anomalously slow spin dynamics to be a common physical property of pyrochlore magnetic materials. The possibility of molecular spin substructures to be associated to the slow dynamics and therefore the short-range correlations is mentioned. The slow spin dynamics observed under field does not exclude the presence of much faster dynamics detected in extremely low or zero field.

  13. Non-Markovian dynamics of a single-mode cavity strongly coupled to an inhomogeneously broadened spin ensemble

    NASA Astrophysics Data System (ADS)

    Krimer, Dmitry O.; Putz, Stefan; Majer, Johannes; Rotter, Stefan

    2014-10-01

    We study the dynamics of a spin ensemble strongly coupled to a single-mode resonator driven by external pulses. When the mean frequency of the spin ensemble is in resonance with the cavity mode, damped Rabi oscillations are found between the spin ensemble and the cavity mode which we describe very accurately, including the dephasing effect of the inhomogeneous spin broadening. We demonstrate that a precise knowledge of this broadening is crucial both for a qualitative and a quantitative understanding of the temporal spin-cavity dynamics. On this basis we show that coherent oscillations between the spin ensemble and the cavity can be enhanced by a few orders of magnitude, when driving the system with pulses that match special resonance conditions. Our theoretical approach is tested successfully with an experiment based on an ensemble of negatively charged nitrogen-vacancy centers in diamond strongly coupled to a superconducting coplanar single-mode waveguide resonator.

  14. Proton-driven spin diffusion in rotating solids via reversible and irreversible quantum dynamics

    PubMed Central

    Veshtort, Mikhail; Griffin, Robert G.

    2011-01-01

    Proton-driven spin diffusion (PDSD) experiments in rotating solids have received a great deal of attention as a potential source of distance constraints in large biomolecules. However, the quantitative relationship between the molecular structure and observed spin diffusion has remained obscure due to the lack of an accurate theoretical description of the spin dynamics in these experiments. We start with presenting a detailed relaxation theory of PDSD in rotating solids that provides such a description. The theory applies to both conventional and radio-frequency-assisted PDSD experiments and extends to the non-Markovian regime to include such phenomena as rotational resonance (R2). The basic kinetic equation of the theory in the non-Markovian regime has the form of a memory function equation, with the role of the memory function played by the correlation function. The key assumption used in the derivation of this equation expresses the intuitive notion of the irreversible dissipation of coherences in macroscopic systems. Accurate expressions for the correlation functions and for the spin diffusion constants are given. The theory predicts that the spin diffusion constants governing the multi-site PDSD can be approximated by the constants observed in the two-site diffusion. Direct numerical simulations of PDSD dynamics via reversible Liouville-von Neumann equation are presented to support and compliment the theory. Remarkably, an exponential decay of the difference magnetization can be observed in such simulations in systems consisting of only 12 spins. This is a unique example of a real physical system whose typically macroscopic and apparently irreversible behavior can be traced via reversible microscopic dynamics. An accurate value for the spin diffusion constant can be usually obtained through direct simulations of PDSD in systems consisting of two 13C nuclei and about ten 1H nuclei from their nearest environment. Spin diffusion constants computed by this method

  15. Immense Magnetic Response of Exciplex Light Emission due to Correlated Spin-Charge Dynamics

    NASA Astrophysics Data System (ADS)

    Wang, Yifei; Sahin-Tiras, Kevser; Harmon, Nicholas J.; Wohlgenannt, Markus; Flatté, Michael E.

    2016-01-01

    As carriers slowly move through a disordered energy landscape in organic semiconductors, tiny spatial variations in spin dynamics relieve spin blocking at transport bottlenecks or in the electron-hole recombination process that produces light. Large room-temperature magnetic-field effects (MFEs) ensue in the conductivity and luminescence. Sources of variable spin dynamics generate much larger MFEs if their spatial structure is correlated on the nanoscale with the energetic sites governing conductivity or luminescence such as in coevaporated organic blends within which the electron resides on one molecule and the hole on the other (an exciplex). Here, we show that exciplex recombination in blends exhibiting thermally activated delayed fluorescence produces MFEs in excess of 60% at room temperature. In addition, effects greater than 4000% can be achieved by tuning the device's current-voltage response curve by device conditioning. Both of these immense MFEs are the largest reported values for their device type at room temperature. Our theory traces this MFE and its unusual temperature dependence to changes in spin mixing between triplet exciplexes and light-emitting singlet exciplexes. In contrast, spin mixing of excitons is energetically suppressed, and thus spin mixing produces comparatively weaker MFEs in materials emitting light from excitons by affecting the precursor pairs. Demonstration of immense MFEs in common organic blends provides a flexible and inexpensive pathway towards magnetic functionality and field sensitivity in current organic devices without patterning the constituent materials on the nanoscale. Magnetic fields increase the power efficiency of unconditioned devices by 30% at room temperature, also showing that magnetic fields may increase the efficiency of the thermally activated delayed fluorescence process.

  16. Dynamics of higher spin gauge fields in AdS d space of dimension d ≥ 5

    NASA Astrophysics Data System (ADS)

    Alkalaev, K. B.

    2006-10-01

    In this overview, the framelike formulation of the dynamics of massless gauge fields of arbitrary spin propagating in Minkowski and (anti-)de Sitter spaces of an arbitrary dimension is discussed. In the framework of the framelike description, the notions of the higher spin field, gauge symmetries and gauge-invariant field strengths are introduced. The general procedure of construction of explicit gauge-invariant action functionals for free higher spin fields is discussed, and some substantial examples of action for fields of particular spins are given. The proposed framelike formulation is an efficient tool for the construction of interaction of higher spin fields on the background of anti-de Sitter geometry. As an example, the nonlinear AdS 5 N = 1 SUSY higher spin field theory describing the interaction of massless higher spin fields between themselves and with gravity in the cubic approximation of action functional is constructed.

  17. First-principles approach to Non-Collinear Magnetism: towards Spin Dynamics

    NASA Astrophysics Data System (ADS)

    Gross, E. K. U.

    2008-03-01

    Most formulations of spin density functional theory (SDFT) restrict the magnetization vector field to have global collinearity. Nevertheless, there exists a wealth of strong non-collinearity in nature, for example molecular magnets, spin-spirals, spin-glasses and all magnets at finite temperatures. The local spin density approximation (LSDA) can be extended to these non-collinear cases [1] but this extension has the undesirable property of having the exchange-correlation (xc) field parallel to the magnetization density at each point in space. When used in conjunction with the equation of motion for the spin magnetization in the absence of spin currents and external fields [2,3], this local collinearity eliminates the torsional term, resulting in no time evolution. This severe shortcoming of LSDA, where the physical prediction is qualitatively wrong, opens up an important new direction for the development of functionals where this time evolution is correctly described. Towards this goal, I will describe our extension of the Kohn-Sham optimized effective potential (OEP) method to the non-collinear case and derive the corresponding integral equations, applicable to both finite and extended systems [3,4]. Most importantly I'll show that the resulting magnetization and xc field are not locally collinear to each other for real solids, and will therefore produce manifestly different spin-dynamics. [1] J. Kuebler, K.-H. Hoeck, J. Sticht and A. R. Williams, J. Phys. F18, 469 (1993). [2] K. Capelle, G. Vignale and B. L. Gyoerffy, Phys. Rev. Lett.87, 206403 (2001). [3] S. Sharma, J. K. Dewhurst, C. Ambrosch-Draxl, S. Kurth, N. Helbig, S. Pittalis, S. Shallcross, L. Nordstroem and E.K.U. Gross Phys. Rev. Lett.98, 196405 (2007) S. Sharma, S. Pittalis, S. Kurth, S. Shallcross, J. K. Dewhurst and E.K.U. Gross Phys. Rev. B76, 100401 (Rapid Comm.) (2007)

  18. Dynamic nuclear polarization assisted spin diffusion for the solid effect case

    NASA Astrophysics Data System (ADS)

    Hovav, Yonatan; Feintuch, Akiva; Vega, Shimon

    2011-02-01

    The dynamic nuclear polarization (DNP) process in solids depends on the magnitudes of hyperfine interactions between unpaired electrons and their neighboring (core) nuclei, and on the dipole-dipole interactions between all nuclei in the sample. The polarization enhancement of the bulk nuclei has been typically described in terms of a hyperfine-assisted polarization of a core nucleus by microwave irradiation followed by a dipolar-assisted spin diffusion process in the core-bulk nuclear system. This work presents a theoretical approach for the study of this combined process using a density matrix formalism. In particular, solid effect DNP on a single electron coupled to a nuclear spin system is considered, taking into account the interactions between the spins as well as the main relaxation mechanisms introduced via the electron, nuclear, and cross-relaxation rates. The basic principles of the DNP-assisted spin diffusion mechanism, polarizing the bulk nuclei, are presented, and it is shown that the polarization of the core nuclei and the spin diffusion process should not be treated separately. To emphasize this observation the coherent mechanism driving the pure spin diffusion process is also discussed. In order to demonstrate the effects of the interactions and relaxation mechanisms on the enhancement of the nuclear polarization, model systems of up to ten spins are considered and polarization buildup curves are simulated. A linear chain of spins consisting of a single electron coupled to a core nucleus, which in turn is dipolar coupled to a chain of bulk nuclei, is considered. The interaction and relaxation parameters of this model system were chosen in a way to enable a critical analysis of the polarization enhancement of all nuclei, and are not far from the values of 13C nuclei in frozen (glassy) organic solutions containing radicals, typically used in DNP at high fields. Results from the simulations are shown, demonstrating the complex dependences of the DNP

  19. New insights into electron spin dynamics in the presence of correlated noise.

    PubMed

    Spezia, S; Adorno, D Persano; Pizzolato, N; Spagnolo, B

    2012-02-01

    The changes in the spin depolarization length in zinc-blende semiconductors when an external component of correlated noise is added to a static driving electric field are analyzed for different values of field strength, noise amplitude and correlation time. Electron dynamics is simulated by a Monte Carlo procedure which takes into account all the possible scattering phenomena of the hot electrons in the medium and includes the evolution of spin polarization. Spin depolarization is studied by examining the decay of the initial spin polarization of the conduction electrons through the D'yakonov-Perel process, the only relevant relaxation mechanism in III-V crystals. Our results show that, for electric field amplitudes lower than the Gunn field, the dephasing length shortens with increasing noise intensity. Moreover, a nonmonotonic behavior of spin depolarization length with the noise correlation time is found, characterized by a maximum variation for values of noise correlation time comparable with the dephasing time. Instead, in high field conditions, we find that, critically depending on the noise correlation time, external fluctuations can positively affect the relaxation length. The influence of the inclusion of the electron-electron scattering mechanism is also shown and discussed.

  20. Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO4

    DOE PAGESBeta

    Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas B. S.; Andersen, Niels H.; Li, Jiying; Le, Manh Duc; Laver, Mark; Niedermayer, Christof; Klemke, Bastian; Lefmann, Kim; et al

    2015-07-06

    We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c. Furthermore, the possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. While using a spin Hamiltonian, we showmore » that the spin dimensionality is intermediate between XY- and Ising-like, with an easy b axis and a hard c axis. As a result, it is shown that both next-nearest neighbor exchange couplings in the bc plane are in competition with the strongest nearest neighbor coupling.« less

  1. Pulse and quench induced dynamical phase transition in a chiral multiferroic spin chain

    NASA Astrophysics Data System (ADS)

    Azimi, M.; Sekania, M.; Mishra, S. K.; Chotorlishvili, L.; Toklikishvili, Z.; Berakdar, J.

    2016-08-01

    Quantum dynamics of magnetic order in a chiral multiferroic chain is studied. We consider two different scenarios: ultrashort terahertz excitations or a sudden electric field quench. Performing analytical and numerical exact diagonalization calculations, we trace the pulse induced spin dynamics and extract quantities that are relevant to quantum information processing. In particular, we analyze the dynamics of the system chirality, the von Neumann entropy, and the pairwise and many-body entanglement. If the characteristic frequencies of the generated states are noncommensurate, then a partial loss of pair concurrence occurs. Increasing the system size, this effect becomes even more pronounced. Many-particle entanglement and chirality are robust and persist in the incommensurate phase. To analyze the dynamical quantum transitions for the quenched and pulsed dynamics we combined the Weierstrass factorization technique for entire functions and the Lanczos exact diagonalization method. For a small system we obtained analytical results including the rate function of the Loschmidt echo. Exact numerical calculations for a system up to 40 spins confirm phase transition. Quench-induced dynamical transitions have been extensively studied recently. Here we show that related dynamical transitions can be achieved and controlled by appropriate electric field pulses.

  2. Tests of Dynamic Scale Model of Gemini Capsule in the Langley 20-Foot Free-Spinning Tunnel

    NASA Technical Reports Server (NTRS)

    1962-01-01

    Tests of Dynamic Scale Model of Gemini Capsule in the Langley 20-Foot Free-Spinning Tunnel. The film shows three spin tunnel tests of a 1/20 scale model of the Gemini capsule. In the first test, the capsule spins freely. In tests 2 and 3, a drogue parachute is attached to the capsule. [Entire movie available on DVD from CASI as Doc ID 20070030989. Contact help@sti.nasa.gov

  3. Quench dynamics of a Bose gas under synthetic spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    Deng, Tian-Shu; Zhang, Wei; Yi, Wei; Guo, Guang-Can; Wei Yi's Group Team; Wei Zhang`s Group Collaboration

    2016-05-01

    We study the quench dynamics of a Bose-Einstein condensate under a Raman-asssited synthetic spin-orbit coupling. To model the dynamical process, we adopt a self-consistent Bogoliubov approach, which is equivalent to applying the time-dependent Bogoliubov-de-Gennes equations. We investigate the dynamics of the condensate fraction as well as the momentum distribution of the Bose gas following a sudden change of system parameters. Typically, the system evolves into a steady state in the long-time limit, which features a stationary condensate fraction and an oscillating momentum distribution. The condensate fraction of the steady state depends on the quench parameter. We investigate how different quench parameters such as the inter- and intra-species interactions and the spin-orbit-coupling parameters affect the condensate fraction in the steady state. Furthermore, we find that the oscillatory momentum distribution in the long-time limit can be described by a generalized Gibbs ensemble with two branches of momentum-dependent Gibbs temperatures. Our study is relevant to the experimental investigation of dynamical processes in a spin-orbit coupled Bose-Einstein condensate.

  4. Quench dynamics of a Bose-Einstein condensate under synthetic spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    Deng, Tian-Shu; Zhang, Wei; Yi, Wei; Guo, Guang-Can

    2016-05-01

    We study the quench dynamics of a Bose-Einstein condensate under a Raman-assisted synthetic spin-orbit coupling. To model the dynamical process, we adopt a self-consistent Bogoliubov approach, which is equivalent to applying the time-dependent Bogoliubov-de Gennes equations. We investigate the dynamics of the condensate fraction as well as the momentum distribution of the Bose gas following a sudden change of system parameters. Typically, the system evolves into a steady state in the long-time limit, which features an oscillating momentum distribution and a stationary condensate fraction. We investigate how different quench parameters such as the inter- and intraspecies interactions and the spin-orbit-coupling parameters affect the condensate fraction in the steady state. Furthermore, we find that the time average of the oscillatory momentum distribution in the long-time limit can be described by a generalized Gibbs ensemble with two branches of momentum-dependent Gibbs temperatures. Our study is relevant to the experimental investigation of dynamical processes in a spin-orbit-coupled Bose-Einstein condensate.

  5. Bifunctional Spin Labeling of Muscle Proteins: Accurate Rotational Dynamics, Orientation, and Distance by EPR.

    PubMed

    Thompson, Andrew R; Binder, Benjamin P; McCaffrey, Jesse E; Svensson, Bengt; Thomas, David D

    2015-01-01

    While EPR allows for the characterization of protein structure and function due to its exquisite sensitivity to spin label dynamics, orientation, and distance, these measurements are often limited in sensitivity due to the use of labels that are attached via flexible monofunctional bonds, incurring additional disorder and nanosecond dynamics. In this chapter, we present methods for using a bifunctional spin label (BSL) to measure muscle protein structure and dynamics. We demonstrate that bifunctional attachment eliminates nanosecond internal rotation of the spin label, thereby allowing the accurate measurement of protein backbone rotational dynamics, including microsecond-to-millisecond motions by saturation transfer EPR. BSL also allows for accurate determination of helix orientation and disorder in mechanically and magnetically aligned systems, due to the label's stereospecific attachment. Similarly, labeling with a pair of BSL greatly enhances the resolution and accuracy of distance measurements measured by double electron-electron resonance (DEER). Finally, when BSL is applied to a protein with high helical content in an assembly with high orientational order (e.g., muscle fiber or membrane), two-probe DEER experiments can be combined with single-probe EPR experiments on an oriented sample in a process we call BEER, which has the potential for ab initio high-resolution structure determination. PMID:26477249

  6. Development of fiber shields for engine containment. [mathematical models

    NASA Technical Reports Server (NTRS)

    Bristow, R. J.; Davidson, C. D.

    1977-01-01

    Tests were conducted in translational launchers and spin pits to generate empirical data used in the design of a Kevlar shield for containing engine burst debris. Methods are given for modeling the relationship of fragment characteristics to shielding requirements. The change in relative importance of shield mounting provisions as fragment energy is increased is discussed.

  7. Imaging Spin Dynamics on the Nanoscale using X-Ray Microscopy

    NASA Astrophysics Data System (ADS)

    Stoll, Hermann; Noske, Matthias; Weigand, Markus; Richter, Kornel; Krüger, Benjamin; Reeve, Robert; Hänze, Max; Adolff, Christian; Stein, Falk-Ulrich; Meier, Guido; Kläui, Mathias; Schütz, Gisela

    2015-04-01

    The dynamics of emergent magnetic quasiparticles, such as vortices, domain walls, and bubbles are studied by scanning transmission x-ray microscopy (STXM), combining magnetic (XMCD) contrast with about 25 nm lateral resolution as well as 70 ps time resolution. Essential progress in the understanding of magnetic vortex dynamics is achieved by vortex core reversal observed by sub-GHz excitation of the vortex gyromode, either by ac magnetic fields or spin transfer torque. The basic switching scheme for this vortex core reversal is the generation of a vortex-antivortex pair. Much faster vortex core reversal is obtained by exciting azimuthal spin wave modes with (multi-GHz) rotating magnetic fields or orthogonal monopolar field pulses in x and y direction, down to 45 ps in duration. In that way unidirectional vortex core reversal to the vortex core 'down' or 'up' state only can be achieved with switching times well below 100 ps. Coupled modes of interacting vortices mimic crystal properties. The individual vortex oscillators determine the properties of the ensemble, where the gyrotropic mode represents the fundamental excitation. By self-organized state formation we investigate distinct vortex core polarization configurations and understand these eigenmodes in an extended Thiele model. Analogies with photonic crystals are drawn. Oersted fields and spin-polarized currents are used to excite the dynamics of domain walls and magnetic bubbles. From the measured phase and amplitude of the displacement of domain walls we deduce the size of the non-adiabatic spin-transfer torque. For sensing applications, the displacement of domain walls is studied and a direct correlation between domain wall velocity and spin structure is found. Finally the synchronous displacement of multiple domain walls using perpendicular field pulses is demonstrated as a possible paradigm shift for magnetic memory and logic applications.

  8. Dynamics of asteroid family halos constrained by spin/shape models

    NASA Astrophysics Data System (ADS)

    Broz, Miroslav

    2016-10-01

    A number of asteroid families cannot be identified solely on the basis of the Hierarchical Clustering Method (HCM), because they have additional 'former' members in the surroundings which constitute a so called halo (e.g. Broz & Morbidelli 2013). They are usually mixed up with the background population which has to be taken into account too.Luckily, new photometric observations allow to derive new spin/shape models, which serve as independent constraints for dynamical models. For example, a recent census of the Eos family shows 43 core and 27 halo asteroids (including background) with known spin orientations.To this point, we present a complex spin-orbital model which includes full N-body dynamics and consequently accounts for all mean-motion, secular, or three-body gravitational resonances, the Yarkovsky drift, YORP effect, collisional reorientations and also spin-orbital interactions. These are especially important for the Koronis family. In this project, we make use of data from the DAMIT database and ProjectSoft Blue Eye 600 observatory.

  9. Dynamics of open quantum spin systems: An assessment of the quantum master equation approach

    NASA Astrophysics Data System (ADS)

    Zhao, P.; De Raedt, H.; Miyashita, S.; Jin, F.; Michielsen, K.

    2016-08-01

    Data of the numerical solution of the time-dependent Schrödinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtaining this quantum master equation, which takes the form of a Bloch equation with time-independent coefficients, accounts for all non-Markovian effects inasmuch the general structure of the quantum master equation allows. Our simulation results show that, with a few rather exotic exceptions, the Bloch-type equation with time-independent coefficients provides a simple and accurate description of the dynamics of a spin-1/2 particle in contact with a thermal bath. A calculation of the coefficients that appear in the Redfield master equation in the Markovian limit shows that this perturbatively derived equation quantitatively differs from the numerically estimated Markovian master equation, the results of which agree very well with the solution of the time-dependent Schrödinger equation.

  10. Dynamics of open quantum spin systems: An assessment of the quantum master equation approach.

    PubMed

    Zhao, P; De Raedt, H; Miyashita, S; Jin, F; Michielsen, K

    2016-08-01

    Data of the numerical solution of the time-dependent Schrödinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtaining this quantum master equation, which takes the form of a Bloch equation with time-independent coefficients, accounts for all non-Markovian effects inasmuch the general structure of the quantum master equation allows. Our simulation results show that, with a few rather exotic exceptions, the Bloch-type equation with time-independent coefficients provides a simple and accurate description of the dynamics of a spin-1/2 particle in contact with a thermal bath. A calculation of the coefficients that appear in the Redfield master equation in the Markovian limit shows that this perturbatively derived equation quantitatively differs from the numerically estimated Markovian master equation, the results of which agree very well with the solution of the time-dependent Schrödinger equation. PMID:27627265

  11. Nonequilibrium dynamics of a mixed spin-1/2 and spin-3/2 Ising ferrimagnetic system with a time dependent oscillating magnetic field source

    NASA Astrophysics Data System (ADS)

    Vatansever, Erol; Polat, Hamza

    2015-10-01

    Nonequilibrium phase transition properties of a mixed Ising ferrimagnetic model consisting of spin-1/2 and spin-3/2 on a square lattice under the existence of a time dependent oscillating magnetic field have been investigated by making use of Monte Carlo simulations with a single-spin flip Metropolis algorithm. A complete picture of dynamic phase boundary and magnetization profiles have been illustrated and the conditions of a dynamic compensation behavior have been discussed in detail. According to our simulation results, the considered system does not point out a dynamic compensation behavior, when it only includes the nearest-neighbor interaction, single-ion anisotropy and an oscillating magnetic field source. As the next-nearest-neighbor interaction between the spins-1/2 takes into account and exceeds a characteristic value which sensitively depends upon values of single-ion anisotropy and only of amplitude of external magnetic field, a dynamic compensation behavior occurs in the system. Finally, it is reported that it has not been found any evidence of dynamically first-order phase transition between dynamically ordered and disordered phases, which conflicts with the recently published molecular field investigation, for a wide range of selected system parameters.

  12. Growth-temperature dependence of optical spin-injection dynamics in self-assembled InGaAs quantum dots

    SciTech Connect

    Yamamura, Takafumi; Kiba, Takayuki; Yang, Xiaojie; Takayama, Junichi; Subagyo, Agus; Sueoka, Kazuhisa; Murayama, Akihiro

    2014-09-07

    The growth-temperature dependence of the optical spin-injection dynamics in self-assembled quantum dots (QDs) of In{sub 0.5}Ga{sub 0.5}As was studied by increasing the sheet density of the dots from 2 × 10{sup 10} to 7 × 10{sup 10} cm{sup −2} and reducing their size through a decrease in growth temperature from 500 to 470 °C. The circularly polarized transient photoluminescence (PL) of the resulting QD ensembles was analyzed after optical excitation of spin-polarized carriers in GaAs barriers by using rate equations that take into account spin-injection dynamics such as spin-injection time, spin relaxation during injection, spin-dependent state-filling, and subsequent spin relaxation. The excitation-power dependence of the transient circular polarization of PL in the QDs, which is sensitive to the state-filling effect, was also examined. It was found that a systematic increase occurs in the degree of circular polarization of PL with decreasing growth temperature, which reflects the transient polarization of exciton spin after spin injection. This is attributed to strong suppression of the filling effect for the majority-spin states as the dot-density of the QDs increases.

  13. Dynamic spin filtering at the Co/Alq3 interface mediated by weakly coupled second layer molecules.

    PubMed

    Droghetti, Andrea; Thielen, Philip; Rungger, Ivan; Haag, Norman; Großmann, Nicolas; Stöckl, Johannes; Stadtmüller, Benjamin; Aeschlimann, Martin; Sanvito, Stefano; Cinchetti, Mirko

    2016-01-01

    Spin filtering at organic-metal interfaces is often determined by the details of the interaction between the organic molecules and the inorganic magnets used as electrodes. Here we demonstrate a spin-filtering mechanism based on the dynamical spin relaxation of the long-living interface states formed by the magnet and weakly physisorbed molecules. We investigate the case of Alq3 on Co and, by combining two-photon photoemission experiments with electronic structure theory, show that the observed long-time spin-dependent electron dynamics is driven by molecules in the second organic layer. The interface states formed by physisorbed molecules are not spin-split, but acquire a spin-dependent lifetime, that is the result of dynamical spin-relaxation driven by the interaction with the Co substrate. Such spin-filtering mechanism has an important role in the injection of spin-polarized carriers across the interface and their successive hopping diffusion into successive molecular layers of molecular spintronics devices. PMID:27578395

  14. Dynamic spin filtering at the Co/Alq3 interface mediated by weakly coupled second layer molecules

    PubMed Central

    Droghetti, Andrea; Thielen, Philip; Rungger, Ivan; Haag, Norman; Großmann, Nicolas; Stöckl, Johannes; Stadtmüller, Benjamin; Aeschlimann, Martin; Sanvito, Stefano; Cinchetti, Mirko

    2016-01-01

    Spin filtering at organic-metal interfaces is often determined by the details of the interaction between the organic molecules and the inorganic magnets used as electrodes. Here we demonstrate a spin-filtering mechanism based on the dynamical spin relaxation of the long-living interface states formed by the magnet and weakly physisorbed molecules. We investigate the case of Alq3 on Co and, by combining two-photon photoemission experiments with electronic structure theory, show that the observed long-time spin-dependent electron dynamics is driven by molecules in the second organic layer. The interface states formed by physisorbed molecules are not spin-split, but acquire a spin-dependent lifetime, that is the result of dynamical spin-relaxation driven by the interaction with the Co substrate. Such spin-filtering mechanism has an important role in the injection of spin-polarized carriers across the interface and their successive hopping diffusion into successive molecular layers of molecular spintronics devices. PMID:27578395

  15. Dynamic spin filtering at the Co/Alq3 interface mediated by weakly coupled second layer molecules.

    PubMed

    Droghetti, Andrea; Thielen, Philip; Rungger, Ivan; Haag, Norman; Großmann, Nicolas; Stöckl, Johannes; Stadtmüller, Benjamin; Aeschlimann, Martin; Sanvito, Stefano; Cinchetti, Mirko

    2016-08-31

    Spin filtering at organic-metal interfaces is often determined by the details of the interaction between the organic molecules and the inorganic magnets used as electrodes. Here we demonstrate a spin-filtering mechanism based on the dynamical spin relaxation of the long-living interface states formed by the magnet and weakly physisorbed molecules. We investigate the case of Alq3 on Co and, by combining two-photon photoemission experiments with electronic structure theory, show that the observed long-time spin-dependent electron dynamics is driven by molecules in the second organic layer. The interface states formed by physisorbed molecules are not spin-split, but acquire a spin-dependent lifetime, that is the result of dynamical spin-relaxation driven by the interaction with the Co substrate. Such spin-filtering mechanism has an important role in the injection of spin-polarized carriers across the interface and their successive hopping diffusion into successive molecular layers of molecular spintronics devices.

  16. Dynamic spin filtering at the Co/Alq3 interface mediated by weakly coupled second layer molecules

    NASA Astrophysics Data System (ADS)

    Droghetti, Andrea; Thielen, Philip; Rungger, Ivan; Haag, Norman; Großmann, Nicolas; Stöckl, Johannes; Stadtmüller, Benjamin; Aeschlimann, Martin; Sanvito, Stefano; Cinchetti, Mirko

    2016-08-01

    Spin filtering at organic-metal interfaces is often determined by the details of the interaction between the organic molecules and the inorganic magnets used as electrodes. Here we demonstrate a spin-filtering mechanism based on the dynamical spin relaxation of the long-living interface states formed by the magnet and weakly physisorbed molecules. We investigate the case of Alq3 on Co and, by combining two-photon photoemission experiments with electronic structure theory, show that the observed long-time spin-dependent electron dynamics is driven by molecules in the second organic layer. The interface states formed by physisorbed molecules are not spin-split, but acquire a spin-dependent lifetime, that is the result of dynamical spin-relaxation driven by the interaction with the Co substrate. Such spin-filtering mechanism has an important role in the injection of spin-polarized carriers across the interface and their successive hopping diffusion into successive molecular layers of molecular spintronics devices.

  17. Dynamic shape effect in {sup 126}Ba at low spin

    SciTech Connect

    Dewald, A.; Weil, D.; Kruecken, R.; Kuehn, R.; Peusquens, R.; Tiesler, H.; Vogel, O.; Zell, K.O.; von Brentano, P.; Bazzacco, D.; Rossi-Alvarez, C.; Pavan, P.; DeAcuna, D.; De Angelis, G.; De Poli, M. ||

    1996-11-01

    Lifetimes of excited states in {sup 126}Ba have been measured with high precision by means of the GASP spectrometer using the coincidence recoil distance technique. The reaction {sup 100}Mo({sup 30}Si,4{ital n}) {sup 126}Ba at a beam energy of 130 MeV was used. The data were analyzed with the differential decay-curve method (DDCM). The obtained transition quadrupole moments disagree with the predictions of the asymmetric rotor model (ARM), the interacting boson model (IBM), and the general collective model (GCM). They give evidence for a sudden dynamic shape change in {sup 126}Ba between the 4{sup +} and 10{sup +} levels of the ground-state band. {copyright} {ital 1996 The American Physical Society.}

  18. Dynamical thermal conductivity of the spin Lieb lattice

    NASA Astrophysics Data System (ADS)

    Yarmohammadi, Mohsen

    2016-05-01

    In the ferromagnetic insulator with the Dzyaloshinskii-Moriya interaction (DMI), we have theoretically investigated the dynamical thermal conductivity (DTC). In other words, we have investigated the frequency dependence of thermal conductivity, κ, of the Lieb lattice, a face-centered square lattice, subjected to a time dependence temperature gradient. Using linear response theory and Green's function approach, DTC has been obtained in the context of Heisenberg Hamiltonian. At low frequencies, DTC is found to be monotonically increasing with DMI strength (DMIS), temperature and next-nearest-neighbor (NNN) coupling. Also we have found that DTC includes a peak for different values of temperature, DMIS and NNN coupling. Furthermore we study the temperature dependence of thermal conductivity of Lieb lattice for different values of DMIS, NNN coupling and external magnetic filed. We witness a decrease in DTC with temperature due to the quantum effects in the system.

  19. Spin Dynamics of a Single Mn Ion in a CdTe/(Cd, Mg, Zn)Te Quantum Dot

    SciTech Connect

    Goryca, Mateusz; Kossacki, Piotr; Golnik, Andrzej; Kazimierczuk, Tomasz; Nawrocki, Michal; Wojnar, Piotr

    2010-01-04

    The spin dynamics of a single Mn ion confined in a CdTe/(Cd, Mg, Zn)Te quantum dot is determined by measurements of photon correlation of photoluminescence. The characteristic time of spin flip is a few nanoseconds and strongly depends on the excitation power.

  20. An efficient numerical method for computing dynamics of spin F = 2 Bose-Einstein condensates

    SciTech Connect

    Wang Hanquan

    2011-07-01

    In this paper, we extend the efficient time-splitting Fourier pseudospectral method to solve the generalized Gross-Pitaevskii (GP) equations, which model the dynamics of spin F = 2 Bose-Einstein condensates at extremely low temperature. Using the time-splitting technique, we split the generalized GP equations into one linear part and two nonlinear parts: the linear part is solved with the Fourier pseudospectral method; one of nonlinear parts is solved analytically while the other one is reformulated into a matrix formulation and solved by diagonalization. We show that the method keeps well the conservation laws related to generalized GP equations in 1D and 2D. We also show that the method is of second-order in time and spectrally accurate in space through a one-dimensional numerical test. We apply the method to investigate the dynamics of spin F = 2 Bose-Einstein condensates confined in a uniform/nonuniform magnetic field.

  1. 1H nuclear spin relaxation of liquid water from molecular dynamics simulations.

    PubMed

    Calero, C; Martí, J; Guàrdia, E

    2015-02-01

    We have investigated the nuclear spin relaxation properties of (1)H in liquid water with the help of molecular dynamics simulations. We have computed the (1)H nuclear spin relaxation times T1 and T2 and determined the contribution of the different interactions to the relaxation at different temperatures and for different classical water models (SPC/E, TIP3P, TIP4P, and TIP4P/2005). Among the water models considered, the TIP4P/2005 model exhibits the best agreement with the experiment. The same analysis was performed with Car-Parrinello ab initio molecular dynamics simulations of bulk water at T = 330 K, which provided results close to the experimental values at room temperature. To complete the study, we have successfully accounted for the temperature-dependence of T1 and T2 in terms of a simplified model, which considers the reorientation in finite angle jumps and the diffusive translation of water molecules.

  2. Spin-lattice dynamics simulation of external field effect on magnetic order of ferromagnetic iron

    SciTech Connect

    Chui, C. P.; Zhou, Yan

    2014-03-15

    Modeling of field-induced magnetization in ferromagnetic materials has been an active topic in the last dozen years, yet a dynamic treatment of distance-dependent exchange integral has been lacking. In view of that, we employ spin-lattice dynamics (SLD) simulations to study the external field effect on magnetic order of ferromagnetic iron. Our results show that an external field can increase the inflection point of the temperature. Also the model provides a better description of the effect of spin correlation in response to an external field than the mean-field theory. An external field has a more prominent effect on the long range magnetic order than on the short range counterpart. Furthermore, an external field allows the magnon dispersion curves and the uniform precession modes to exhibit magnetic order variation from their temperature dependence.

  3. Dynamical modelling and control of a spacecraft-mounted manipulator capturing a spinning satellite

    NASA Astrophysics Data System (ADS)

    Cyril, Xavier; Jaar, Gilbert J.; Misra, Arun K.

    1995-01-01

    Issues associated with the modelling and control of a spacecraft-mounted manipulator capturing a spinning satellite are presented. The Lagrangian formulation is used to derive the dynamical equations of the system immediately following the capture. The formulation is carried out by writing Lagrange's equations for the individual bodies, and then assembling them to obtain the constrained dynamical equations of the system. The non-working constraint forces/torques are then eliminated by using the natural orthogonal complement which produces a set of independent dynamical equations. A control algorithm whose objective is to produce a set of feedback-linearized, homogeneous and uncoupled equations is designed and implemented. The initial conditions of the state variables needed to achieve smooth berthing of the satellite are computed, and the dynamics simulation of both the controlled and uncontrolled systems is carried out. The manipulator's structural flexibility is included in the dynamics simulation model.

  4. The dynamics of diluted Ho spin ice Ho2-xYxTi2O7 studied byneutron spin echo spectroscopy

    SciTech Connect

    Ehlers, G.; Gardner, J.S.; Booth, C.H.; Daniel, M.; Kam, K.C.; Cheetham, A.K.; Antonio, D.; Brooks, H.E.; Cornelius, A.L.; Bramwell,S.T.; Lago, J.; Haussler, W.; Rosov, N.

    2006-02-27

    We have studied the spin relaxation in diluted spin ice Ho{sub 2-x} Y{sub x} Ti{sub 2}O{sub 7} by means of neutron spin echo spectroscopy. Remarkably, the geometrical frustration is not relieved by doping with non-magnetic Y, and the dynamics of the freezing is unaltered in the spin echo time window up to x {approx_equal} 1.6. At higher doping with non-magnetic Y (x {ge} 1.6) a new relaxation process at relatively high temperature (up to at least T {approx_equal} 55 K) appears which is more than 10 times faster than the thermally activated main relaxation process. We find evidence that over the whole range of composition all Ho spins participate in the dynamics. These results are compared to a.c. susceptibility measurements of the diluted Ho and Dy spin ice systems. X-ray absorption fine structure (EXAFS) spectra and x-ray diffraction show that the samples are structurally well ordered.

  5. Dynamics and supramolecular organization of the 1D spin transition polymeric chain compound [Fe(NH2trz)3](NO3)2. Muon spin relaxation.

    PubMed

    Garcia, Yann; Campbell, Stewart J; Lord, James S; Boland, Yves; Ksenofontov, Vadim; Gütlich, Philipp

    2007-09-27

    The thermal spin transition that occurs in the polymeric chain compound [Fe(NH(2)trz)3](NO3)2 above room temperature has been investigated by zero-field muon spin relaxation (microSR) over the temperature range approximately 8-402 K. The depolarization curves are best described by a Lorentzian and a Gaussian line that represent fast and slow components, respectively. The spin transition is associated with a hysteresis loop of width DeltaT = 34 K (T1/2 upward arrow = 346 K and T1/2 downward arrow = 312 K) that has been delineated by the temperature variation of the initial asymmetry parameter, in good agreement with previously published magnetic measurements. Zero-field and applied field (20-2000 Oe) microSR measurements show the presence of diamagnetic muon species and paramagnetic muonium radical species (A = 753 +/- 77 MHz) over the entire temperature range. Fast dynamics have been revealed in the high-spin state of [Fe(NH(2)trz)3](NO3)2 with the presence of a Gaussian relaxation mode that is mostly due to the dipolar interaction with static nuclear moments. This situation, where the muonium radicals are totally decoupled and not able to sense paramagnetic fluctuations, implies that the high-spin dynamics fall outside the muon time scale. Insights to the origin of the cooperative effects associated with the spin transition of [Fe(NH(2)trz)3](NO3)2 through muon implantation are presented.

  6. Rapid 3D dynamic arterial spin labeling with a sparse model-based image reconstruction.

    PubMed

    Zhao, Li; Fielden, Samuel W; Feng, Xue; Wintermark, Max; Mugler, John P; Meyer, Craig H

    2015-11-01

    Dynamic arterial spin labeling (ASL) MRI measures the perfusion bolus at multiple observation times and yields accurate estimates of cerebral blood flow in the presence of variations in arterial transit time. ASL has intrinsically low signal-to-noise ratio (SNR) and is sensitive to motion, so that extensive signal averaging is typically required, leading to long scan times for dynamic ASL. The goal of this study was to develop an accelerated dynamic ASL method with improved SNR and robustness to motion using a model-based image reconstruction that exploits the inherent sparsity of dynamic ASL data. The first component of this method is a single-shot 3D turbo spin echo spiral pulse sequence accelerated using a combination of parallel imaging and compressed sensing. This pulse sequence was then incorporated into a dynamic pseudo continuous ASL acquisition acquired at multiple observation times, and the resulting images were jointly reconstructed enforcing a model of potential perfusion time courses. Performance of the technique was verified using a numerical phantom and it was validated on normal volunteers on a 3-Tesla scanner. In simulation, a spatial sparsity constraint improved SNR and reduced estimation errors. Combined with a model-based sparsity constraint, the proposed method further improved SNR, reduced estimation error and suppressed motion artifacts. Experimentally, the proposed method resulted in significant improvements, with scan times as short as 20s per time point. These results suggest that the model-based image reconstruction enables rapid dynamic ASL with improved accuracy and robustness.

  7. Quantum jumps and spin dynamics of interacting atoms in a strongly coupled atom-cavity system.

    PubMed

    Khudaverdyan, M; Alt, W; Kampschulte, T; Reick, S; Thobe, A; Widera, A; Meschede, D

    2009-09-18

    We experimentally investigate the spin dynamics of one and two neutral atoms strongly coupled to a high finesse optical cavity. We observe quantum jumps between hyperfine ground states of a single atom. The interaction-induced normal-mode splitting of the atom-cavity system is measured via the atomic excitation. Moreover, we observe the mutual influence of two atoms simultaneously coupled to the cavity mode.

  8. Discrimination of nuclear spin isomers exploiting the excited state dynamics of a quinodimethane derivative

    SciTech Connect

    Obaid, Rana; Kinzel, Daniel; Oppel, Markus González, Leticia

    2014-10-28

    Despite the concept of nuclear spin isomers (NSIs) exists since the early days of quantum mechanics, only few approaches have been suggested to separate different NSIs. Here, a method is proposed to discriminate different NSIs of a quinodimethane derivative using its electronic excited state dynamics. After electronic excitation by a laser field with femtosecond time duration, a difference in the behavior of several quantum mechanical operators can be observed. A pump-probe experimental approach for separating these different NSIs is then proposed.

  9. Lattice dynamics and spin-phonon interactions in multiferroic RMn2O5: Shell model calculations

    NASA Astrophysics Data System (ADS)

    Litvinchuk, A. P.

    2009-08-01

    The results of the shell model lattice dynamics calculations of multiferroic RMn2O5 materials (space group Pbam) are reported. Theoretical even-parity eigenmode frequencies are compared with those obtained experimentally in polarized Raman scattering experiments for R=Ho,Dy. Analysis of displacement patterns allows to identify vibrational modes which facilitate spin-phonon coupling by modulating the Mn-Mn exchange interaction and provides explanation of the observed anomalous temperature behavior of phonons.

  10. RVB signatures in the spin dynamics of the square-lattice Heisenberg antiferromagnet

    NASA Astrophysics Data System (ADS)

    Ghioldi, E. A.; Gonzalez, M. G.; Manuel, L. O.; Trumper, A. E.

    2016-03-01

    We investigate the spin dynamics of the square-lattice spin-\\frac{1}{2} Heisenberg antiferromagnet by means of an improved mean-field Schwinger boson calculation. By identifying both, the long-range Néel and the RVB-like components of the ground state, we propose an educated guess for the mean-field magnetic excitation consisting on a linear combination of local and bond spin flips to compute the dynamical structure factor. Our main result is that when this magnetic excitation is optimized in such a way that the corresponding sum rule is fulfilled, we recover the low- and high-energy spectral weight features of the experimental spectrum. In particular, the anomalous spectral weight depletion at (π,0) found in recent inelastic neutron scattering experiments can be attributed to the interference of the triplet bond excitations of the RVB component of the ground state. We conclude that the Schwinger boson theory seems to be a good candidate to adequately interpret the dynamic properties of the square-lattice Heisenberg antiferromagnet.

  11. Bioengineering Spin-Offs from Dynamical Systems Theory

    NASA Astrophysics Data System (ADS)

    Collins, J. J.

    1997-03-01

    Recently, there has been considerable interest in applying concepts and techniques from dynamical systems and statistical physics to physiological systems. In this talk, we present work dealing which two active topics in this area: stochastic resonance and (2) chaos control. Stochastic resonance is a phenomenon wherein the response of nonlinear system to a weak input signal is optimally enhanced by the presence of a particular level of noise. Here we demonstrate that noise-based techniques can be used to lower sensory detection thresholds in humans. We discuss how from a bioengineering and clinical standpoint, these developments may be particularly relevant for individuals with elevated sensory thresholds, such as older adults and patients with peripheral neuropathy. Chaos control techniques have been applied to a wide range of experimental systems, including biological preparations. The application of chaos control to biological systems has led to speculations that these methods may be clinically useful. Here we demonstrate that the principles of chaos control can be utilized to stabilize underlying unstable periodic orbits in non-chaotic biological systems. We discuss how from a bioengineering and clinical standpoint, these developments may be important for suppressing or eliminating certain types of cardiac arrhythmias.

  12. First glimpse of the soft x-ray induced excited spin-state trapping effect dynamics on spin cross-over molecules

    SciTech Connect

    Davesne, V.; Gruber, M.; Miyamachi, T.; Da Costa, V.; Boukari, S.; Scheurer, F.; Joly, L.; Bowen, M.; Beaurepaire, E.; Ohresser, P.; Otero, E.; Choueikani, F.; Gaspar, A. B.; Real, J. A.; Wulfhekel, W.

    2013-08-21

    The dynamics of the soft x-ray induced excited spin state trapping (SOXIESST) effect of Fe(phen){sub 2}(NCS){sub 2} (Fe-phen) powder have been investigated by x-ray absorption spectroscopy (XAS) using the total electron yield method, in a wide temperature range. The low-spin (LS) state is excited into the metastable high-spin (HS) state at a rate that depends on the intensity of the x-ray illumination it receives, and both the temperature and the intensity of the x-ray illumination will affect the maximum HS proportion that is reached. We find that the SOXIESST HS spin state transforms back to the LS state at a rate that is similar to that found for the light induced excited spin state trapping (LIESST) effect. We show that it is possible to use the SOXIESST effect in combination with the LIESST effect to investigate the influence of cooperative behavior on the dynamics of both effects. To investigate the impact of molecular cooperativity, we compare our results on Fe-phen with those obtained for Fe([Me{sub 2}Pyrz]{sub 3}BH){sub 2} (Fe-pyrz) powder, which exhibits a similar thermal transition temperature but with a hysteresis. We find that, while the time constant of the dynamic is identical for both molecules, the SOXIESST effect is less efficient at exciting the HS state in Fe-pyrz than in Fe-phen.

  13. Spin-wave dynamics of magnetic heterostructures: Application to Dy/Y multilayers

    SciTech Connect

    Haraldsen, Jason T; Fishman, Randy Scott

    2010-01-01

    We examine the spin-wave (SW) dynamics of Dy/Y multilayers in order to separate the dynamical contribution of the Dy-Y interface from that of bulk Dy. The SW frequencies and intensities of bulk Dy are determined analytically. When the Dy layers in a multilayer geometry are decoupled, the SW dispersion relations are discontinuous with discrete excitations. With a RKKY interaction coupling through the Y spacer, the discrete excitations become dispersive and the main SW branches split due to the multilayer geometry. Regardless of the strength of the intermediate RKKY interaction, the dispersion signature of the bulk remains.

  14. Probing dynamics of fusion reactions through cross-section and spin distribution measurement

    NASA Astrophysics Data System (ADS)

    Kaur, Maninder; Behera, B. R.; Singh, Gulzar; Singh, Varinderjit; Madhavan, N.; Muralithar, S.; Nath, S.; Gehlot, J.; Mohanto, G.; Mukul, Ish; Siwal, D.; Thakur, M.; Kapoor, K.; Sharma, P.; Banerjee, T.; Jhingan, A.; Varughese, T.; Bala, Indu; Nayak, B. K.; Saxena, A.; Chatterjee, M. B.; Stevenson, P. D.

    2016-05-01

    Present work aims to explicate the effect of entrance channel mass asymmetry on fusion dynamics for the Compound Nucleus 80Sr populated through two different channels, 16O+64Zn and 32S+48Ti, using cross-section and spin distribution measurements as probes. The evaporation spectra studies for these systems, reported earlier indicate the presence of dynamical effects for mass symmetric 32S+48Ti system.The CCDEF and TDHF calculations have been performed for both the systems and an attempt has been made to explain the reported deviations in the α-particle spectrum for the mass symmetric system.

  15. Energy Band and Josephson Dynamics of Spin-Orbit Coupled Bose-Einstein Condensates

    NASA Astrophysics Data System (ADS)

    Zhang, Xin; Yu, Zi-Fa; Xue, Ju-Kui

    2015-10-01

    We theoretically investigate the energy band structure and Josephson dynamics of a spin-orbit coupled Bose-Einstein condensate in a double-well potential. We study the energy band structure and the corresponding tunneling dynamics of the system by properly adjusting the SO coupling, Raman coupling, Zeeman field and atomic interactions. The coupled effects of SO coupling, Raman coupling, Zeeman field and atomic interactions lead to the appearance of complex energy band structure including the loop structure. Particularly, the emergence of the loop structure in energy band also depends on SO coupling, Raman coupling, Zeeman field and atomic interactions. Correspondingly, the Josephson dynamics of the system are strongly related to the energy band structure. Especially, the emergence of the loop structure results in complex tunneling dynamics, including suppression-revival transitions and self-trapping of atoms transfer between two spin states and two wells. This engineering provides a possible means for studying energy level and corresponding dynamics of two-species SO coupled BECs. Supported by the National Natural Science Foundation of China under Grant Nos. 11274255 and 11305132, by Specialized Research Fund for the Doctoral Program of Higher Education of China under Grant No. 20136203110001, by the Natural Science Foundation of Gansu province under Grant No. 2011GS04358, and by Creation of Science and Technology of Northwest Normal University under Grant Nos. NWNU-KJCXGC-03-48, NWNU-LKQN-12-12

  16. Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer.

    PubMed

    Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent

    2016-01-01

    Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers. PMID:27425776

  17. Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer

    NASA Astrophysics Data System (ADS)

    Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J.; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent

    2016-07-01

    Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers.

  18. Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer

    PubMed Central

    Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent

    2016-01-01

    Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers. PMID:27425776

  19. Simultaneous resolution of the micromagnetic and spin transport equations applied to current-induced domain wall dynamics

    NASA Astrophysics Data System (ADS)

    Sturma, M.; Bellegarde, C.; Toussaint, J.-C.; Gusakova, D.

    2016-09-01

    In this paper, we use simulations to study current-induced domain wall dynamics by simultaneously resolving the spin transport and micromagnetic equations for a three-dimensional ferromagnetic strip. In contrast to local approaches, which neglect mutual interaction between spins and magnetic moments, our approach recalculates the spin distribution at each time step using the generalized drift diffusion model, which takes the transverse spin absorption phenomenon into account. We quantified the differences between a local approach and treatment based on a self-consistent method by plotting the domain wall velocity as a function of the domain wall width. We also characterized the domain wall velocity and the Walker breakdown condition as a function of the transverse spin absorption length l⊥, which plays a crucial role in domain wall dynamics.

  20. A spinning thermometer to monitor microwave heating and glass transitions in dynamic nuclear polarization.

    PubMed

    Miéville, Pascal; Vitzthum, Veronika; Caporini, Marc A; Jannin, Sami; Gerber-Lemaire, Sandrine; Bodenhausen, Geoffrey

    2011-11-01

    As previously demonstrated by Thurber and Tycko, the peak position of (79)Br in potassium bromide (KBr) allows one to determine the temperature of a spinning sample. We propose to adapt the original design by using a compact KBr tablet placed at the bottom of the magic angle spinning rotor, separated from the sample under investigation by a thin disk made of polytetrafluoroethylene (or 'Teflon'®). This design allows spinning the sample up to at least 16 kHz. The KBr tablet can remain in the rotor when changing the sample under investigation. Calibration in the range of 98 < T < 320 K has been carried out in a static rotor by inserting a platinum thermometer. The accuracy is better than ± 0.9 K, even in the presence of microwave irradiation. Irradiation with 5 W microwaves at 263 GHz leads to a small temperature increase of 3.6 ± 1.4 K in either static or spinning samples. The dynamic nuclear polarization enhancement decreases with increasing temperature, in particular when a frozen glassy sample undergoes a glass transition.

  1. Minority-spin dynamics in the nonhomogeneous Ising model: Diverging time scales and exponents

    NASA Astrophysics Data System (ADS)

    Mullick, Pratik; Sen, Parongama

    2016-05-01

    We investigate the dynamical behavior of the Ising model under a zero-temperature quench with the initial fraction of up spins 0 ≤x ≤1 . In one dimension, the known results for persistence probability are verified; it shows algebraic decay for both up and down spins asymptotically with different exponents. It is found that the conventional finite-size scaling is valid here. In two dimensions, however, the persistence probabilities are no longer algebraic; in particular for x ≤0.5 , persistence for the up (minority) spins shows the behavior Pmin(t ) ˜t-γexp[-(t/τ ) δ] with time t , while for the down (majority) spins, Pmaj(t ) approaches a finite value. We find that the timescale τ diverges as (xc-x ) -λ, where xc=0.5 and λ ≃2.31 . The exponent γ varies as θ2 d+c0(xc-x ) β where θ2 d≃0.215 is very close to the persistence exponent in two dimensions; β ≃1 . The results in two dimensions can be understood qualitatively by studying the exit probability, which for different system size is found to have the form E (x ) =f [(x/-xc xc) L1 /ν] , with ν ≈1.47 . This result suggests that τ ˜Lz ˜ , where z ˜=λ/ν =1.57 ±0.11 is an exponent not explored earlier.

  2. Dynamics of a coupled spin-vortex pair in dipolar spinor Bose-Einstein condensates

    NASA Astrophysics Data System (ADS)

    Li, Tiantian; Yi, Su; Zhang, Yunbo

    2016-05-01

    The collisional and magnetic field quench dynamics of a coupled spin-vortex pair in dipolar spinor Bose-Einstein condensates in a double-well potential are numerically investigated in the mean-field theory. Upon a sudden release of the potential barrier the two layers of condensates collide with each other in the trap center with the chirality of the vortex pair exchanged after each collision, showing the typical signature of in-phase collision for the parallel spin-vortex phase, and out-of-phase collision for the antiparallel phase. When quenching the transverse magnetic field, the vortex center in the single-layered condensate starts to make a helical motion with oval-shaped trajectories and the displacement of the center position is found to exhibit a damped simple harmonic oscillation with an intrinsic frequency and damping rate. The oscillation mode of the spin-vortex pair may be tuned by the initial magnetic field and the height of the Gaussian barrier; e.g., the gyrotropic motions for a parallel spin-vortex pair are out of sync with each other in the two layers, while those for the antiparallel pair exhibit a double-helix structure with the vortex centers moving opposite to each other with the same amplitude.

  3. Evidence of impurity and boundary effects on magnetic monopole dynamics in spin ice

    NASA Astrophysics Data System (ADS)

    Revell, H. M.; Yaraskavitch, L. R.; Mason, J. D.; Ross, K. A.; Noad, H. M. L.; Dabkowska, H. A.; Gaulin, B. D.; Henelius, P.; Kycia, J. B.

    2013-01-01

    Electrical resistance is a crucial and well-understood property of systems ranging from computer microchips to nerve impulse propagation in the human body. Here we study the motion of magnetic charges in spin ice and find that extra spins inserted in Dy2Ti2O7 trap magnetic monopole excitations and provide the first example of how defects in a spin-ice material obstruct the flow of monopoles--a magnetic version of residual resistance. We measure the time-dependent magnetic relaxation in Dy2Ti2O7 and show that it decays with a stretched exponential followed by a very slow long-time tail. In a Monte Carlo simulation governed by Metropolis dynamics we show that surface effects and a very low level of stuffed spins (0.30%)--magnetic Dy ions substituted for non-magnetic Ti ions--cause these signatures in the relaxation. In addition, we find evidence that the rapidly diverging experimental timescale is due to a temperature-dependent attempt rate proportional to the monopole density.

  4. Detection of topological states in two-dimensional Dirac systems by the dynamic spin susceptibility

    NASA Astrophysics Data System (ADS)

    Nakamura, Masaaki; Tokuno, Akiyuki

    2016-08-01

    We discuss dynamic spin susceptibility (DSS) in two-dimensional (2D) Dirac electrons with spin-orbit interactions to characterize topological insulators. The imaginary part of the DSS appears as an absorption rate in response to a transverse ac magnetic field, just as in an electron spin resonance experiment for localized spin systems. We found that when the system is in a static magnetic field, the topological state can be identified by an anomalous resonant peak of the imaginary part of the DSS as a function of the frequency of the transverse magnetic field ω . In the absence of a static magnetic field, the imaginary part of the DSS becomes a continuous function of ω with a threshold frequency ωc. In this case, the topological and the trivial phases can also be distinguished by the values of ωc and by the line shapes. Thus the DSS is an experimentally observable physical quantity to characterize a topological insulator directly from bulk properties, without observing a topological transition.

  5. Detection of topological states in two-dimensional Dirac systems by the dynamic spin susceptibility

    NASA Astrophysics Data System (ADS)

    Nakamura, Masaaki; Tokuno, Akiyuki

    We discuss dynamic spin susceptibility (DSS) in two-dimensional (2D) Dirac electrons with spin-orbit interactions to characterize topological insulators. The imaginary part of the DSS appears as an absorption rate in response to a transverse AC magnetic field, just like an electron spin resonance experiment for localized spin systems. We found that when the system is in a static magnetic field, the topological state can be identified by an anomalous resonant peak of the imaginary part of the DSS as a function of the frequency of the transverse magnetic field ω. This anomalous peak is related to a transition between two Landau levels close to the Fermi level, which is not allowed in the trivial state. In the absence of the static magnetic field, the imaginary part of the DSS becomes a continuous function of ω with a threshold frequency ωc. In this case, the topological and the trivial phases can also be distinguished by the values of ωc and by the line shapes. Thus the DSS is an essential and an experimentally observable physical quantity to characterize the topological insulators.

  6. Dynamic field-frequency lock for tracking magnetic field fluctuations in electron spin resonance experiments

    NASA Astrophysics Data System (ADS)

    Asfaw, Abraham; Tyryshkin, Alexei; Lyon, Stephen

    Global magnetic field fluctuations present significant challenges to pulsed electron spin resonance experiments on systems with long spin coherence times. We will discuss results from experiments in which we follow instantaneous changes in magnetic field by locking to the free induction decay of a proton NMR signal using a phase-locked loop. We extend conventional field-frequency locking techniques used in NMR to follow slow magnetic field drifts by using a modified Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence in which the phase of the pi-pulses follows the phase of the proton spins at all times. Hence, we retain the ability of the CPMG pulse sequence to refocus local magnetic field inhomogeneities without refocusing global magnetic field fluctuations. In contrast with conventional field-frequency locking techniques, our experiments demonstrate the potential of this method to dynamically track global magnetic field fluctuations on timescales of about 2 seconds and with rates faster than a kHz. This frequency range covers the dominant noise frequencies in our electron spin resonance experiments as previously reported.

  7. Improving the coherence properties of solid-state spin ensembles via optimized dynamical decoupling

    NASA Astrophysics Data System (ADS)

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2016-04-01

    In this work, we optimize a dynamical decoupling (DD) protocol to improve the spin coherence properties of a dense ensemble of nitrogen-vacancy (NV) centers in diamond. Using liquid nitrogen-based cooling and DD microwave pulses, we increase the transverse coherence time T2 from ˜ 0.7 ms up to ˜ 30 ms. We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. After performing a detailed analysis of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the concatenated XY8 pulse sequences serves as the optimal control scheme for preserving an arbitrary spin state. Finally, we use the concatenated sequences to demonstrate an immediate improvement of the AC magnetic sensitivity up to a factor of two at 250 kHz. For future work, similar protocols may be used to increase coherence times up to NV-NV interaction time scales, a major step toward the creation of quantum collective NV spin states.

  8. Direct observation of magnetization dynamics generated by nanocontact spin-torque vortex oscillators

    NASA Astrophysics Data System (ADS)

    Keatley, P. S.; Sani, S. R.; Hrkac, G.; Mohseni, S. M.; Dürrenfeld, P.; Loughran, T. H. J.; Åkerman, J.; Hicken, R. J.

    2016-08-01

    Time-resolved scanning Kerr microscopy has been used to directly image the magnetization dynamics of nanocontact (NC) spin-torque vortex oscillators (STVOs) when phase locked to an injected microwave (rf) current. The Kerr images reveal free-layer magnetization dynamics that extend outside the NC footprint, where they cannot be detected electrically, but which are crucial to phase-lock STVOs that share common magnetic layers. For a single NC, dynamics were observed not only when the STVO frequency was fully locked to that of the rf current, but also for a partially locked state characterized by periodic changes in the core trajectory at the rf frequency. For a pair of NCs, we explore the correlation between the spatial character of injection-locked dynamics and the free-running spectra. Insight gained from these images may improve understanding of the conditions required for mutual phase locking of multiple STVOs, and hence enhanced microwave power emission.

  9. Debye Shielding

    NASA Astrophysics Data System (ADS)

    Jones, Robert

    2011-10-01

    We usually expect that a biased electrode in contact with a plasma will effect only its immediate surroundings. The plasma will tend to shield itself from the applied electric potential, the characteristic shielding distance being the Debye length. This is not the case for biased gun electrodes which can project a nonneutral plasma beam relatively long distances across a magnetically confined plasma (Controlling the plasma potential across a magnetic field, Trans. Kansas Acad. Sci., vol 93, pg 125, R. Jones, 1990 and Plasma heating with electrically biased plasma guns, Trans. Kansas Acad. Sci., vol 97, pg 136, R. Jones, 1994) See also my website www.robert-w-jones.com and blog www.robertwilliamjones.blogspot.com.

  10. Time-resolved x-ray imaging of magnetization dynamics in spin-transfer torque devices

    SciTech Connect

    Chembrolu, V.

    2010-02-24

    Time-resolved x-ray imaging techniques have recently demonstrated the capability to probe the magnetic switching of nanoscale devices. This technique has enabled, for example, the direct observation of the nonuniform intermediate states assumed by the magnetic free layer during reversal by a spin-polarized current. These experiments have shown an interesting size-dependent behavior associated with the motion of vortices to mediate the magnetization reversal which cannot be explained by the macrospin picture of spin-torque switching. In this paper we present both experimental and analytical results which show the origin of the complex switching behavior. We use time-resolved x-ray microscopy to further study the switching behavior of samples with 45{sup o} angle between the free and polarizing magnetic layers. A model is developed in terms of a linearized Landau-Lifshitz-Gilbert equation showing that the initial dynamics is dominated by the balance between the Oersted field and thermal fluctuations. The spin torque amplifies this dynamics, leading to a strong sensitivity to sample size, angle, and temperature. The model is in good agreement with current and previous experimental observations.

  11. Quantum spin dynamics and entanglement in systems with long-range interactions

    NASA Astrophysics Data System (ADS)

    Rey, Ana M.

    One of the fundamental goals of modern quantum sciences is to learn how to control and manipulate non-equilibrium many-body systems and use them to make powerful and improved quantum devices, materials and technologies. However, out-of-equilibrium systems are complex, typically strongly correlated and entangled, and thus to model them we are in an urgent need of new methodologies. In this talk I will discuss new theoretical methods that we have developed to investigate emergent non-equilibrium phenomena in driven-dissipative spin systems interacting via long-range interactions. I will show we can capture the dynamics of correlations and entanglement in close systems and the interplay between dissipation and entanglement in open quantum systems including spin-boson models. As a specific application I will discuss the use of our methods to model the spin dynamics exhibited by arrays of trapped ions with controllable long-range interactions. I will show that our predictions are consistent with recent experimental measurements. I will also discuss new protocols to diagnostic and characterize entanglement based on well-established NMR protocols This work is supported by NSF, ARO, AFOSR-MURI, and NIST.

  12. Tracking protein dynamics with photoconvertible Dendra2 on spinning disk confocal systems.

    PubMed

    Woods, Elena; Courtney, Jane; Scholz, Dimitri; Hall, William W; Gautier, Virginie W

    2014-12-01

    Understanding the dynamic properties of cellular proteins in live cells and in real time is essential to delineate their function. In this context, we introduce the Fluorescence Recovery After Photobleaching-Photoactivation unit (Andor) combined with the Nikon Eclipse Ti E Spinning Disk (Andor) confocal microscope as an advantageous and robust platform to exploit the properties of the Dendra2 photoconvertible fluorescent protein (Evrogen) and analyse protein subcellular trafficking in living cells. A major advantage of the spinning disk confocal is the rapid acquisition speed, enabling high temporal resolution of cellular processes. Furthermore, photoconversion and imaging are less invasive on the spinning disk confocal as the cell exposition to illumination power is reduced, thereby minimizing photobleaching and increasing cell viability. We have tested this commercially available platform using experimental settings adapted to track the migration of fast trafficking proteins such as UBC9, Fibrillarin and have successfully characterized their differential motion between subnuclear structures. We describe here step-by-step procedures, with emphasis on cellular imaging parameters, to successfully perform the dynamic imaging and photoconversion of Dendra2-fused proteins at high spatial and temporal resolutions necessary to characterize the trafficking pathways of proteins.

  13. Nanocluster building blocks of artificial square spin ice: Stray-field studies of thermal dynamics

    SciTech Connect

    Pohlit, Merlin Porrati, Fabrizio; Huth, Michael; Müller, Jens

    2015-05-07

    We present measurements of the thermal dynamics of a Co-based single building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition. We employ micro-Hall magnetometry, an ultra-sensitive tool to study the stray field emanating from magnetic nanostructures, as a new technique to access the dynamical properties during the magnetization reversal of the spin-ice nanocluster. The obtained hysteresis loop exhibits distinct steps, displaying a reduction of their “coercive field” with increasing temperature. Therefore, thermally unstable states could be repetitively prepared by relatively simple temperature and field protocols allowing one to investigate the statistics of their switching behavior within experimentally accessible timescales. For a selected switching event, we find a strong reduction of the so-prepared states' “survival time” with increasing temperature and magnetic field. Besides the possibility to control the lifetime of selected switching events at will, we find evidence for a more complex behavior caused by the special spin ice arrangement of the macrospins, i.e., that the magnetic reversal statistically follows distinct “paths” most likely driven by thermal perturbation.

  14. Kinematical and dynamical aspects of higher-spin bound-state equations in holographic QCD

    SciTech Connect

    de Téramond, Guy F.; Dosch, Hans Günter; Brodsky, Stanley J.

    2013-04-01

    In this paper we derive holographic wave equations for hadrons with arbitrary spin starting from an effective action in a higher-dimensional space asymptotic to anti–de Sitter (AdS) space. Our procedure takes advantage of the local tangent frame, and it applies to all spins, including half-integer spins. An essential element is the mapping of the higher-dimensional equations of motion to the light-front Hamiltonian, thus allowing a clear distinction between the kinematical and dynamical aspects of the holographic approach to hadron physics. Accordingly, the nontrivial geometry of pure AdS space encodes the kinematics, and the additional deformations of AdS space encode the dynamics, including confinement. It thus becomes possible to identify the features of holographic QCD, which are independent of the specific mechanisms of conformal symmetry breaking. In particular, we account for some aspects of the striking similarities and differences observed in the systematics of the meson and baryon spectra.

  15. Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings.

    PubMed

    Vedmedenko, E Y

    2016-02-19

    Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed. PMID:26943555

  16. Collective dynamics of a spin-orbit-coupled Bose-Einstein condensate.

    PubMed

    Hu, Fang-Qi; Wang, Jian-Jun; Yu, Zi-Fa; Zhang, Ai-Xia; Xue, Ju-Kui

    2016-02-01

    We study the collective dynamics of the spin-orbit coupled two pseudospin components of a Bose-Einstein condensate trapped in a quasi-one-dimensional harmonic potential, by using variational and directly numerical approach of binary mean-field Gross-Pitaevskii equations. The results show that, because of strong coupling of spin-orbit coupling (SOC), Rabi coupling, and atomic interaction, the collective dynamics of the system behave as complex characters. When the Rabi coupling is absent, the density profiles of the system preserve the Gauss type and the wave packets do harmonic oscillations. The amplitude of the collective oscillations increases with SOC. Furthermore, when the SOC strength increases, the dipole oscillations of the two pseudospin components undergo a transition from in-phase to out-of-phase oscillations. When the Rabi coupling present, there will exist a critical value of SOC strength (which depends on the Rabi coupling and atomic interaction). If the SOC strength is less than this critical value, the density profiles of the system can preserve the Gauss type and the wave packets do anharmonic (the frequency of dipole oscillations depends on SOC) oscillations synchronously (i.e., in-phase oscillations). However, if the SOC strength is larger than this critical value, the wave packets are dynamically fragmented and the stable dipole oscillations of the system can not exist. The collective dynamics of the system can be controlled by adjusting the atomic interaction, SOC, and Rabi-coupling strength.

  17. Collective dynamics of a spin-orbit-coupled Bose-Einstein condensate

    NASA Astrophysics Data System (ADS)

    Hu, Fang-Qi; Wang, Jian-Jun; Yu, Zi-Fa; Zhang, Ai-Xia; Xue, Ju-Kui

    2016-02-01

    We study the collective dynamics of the spin-orbit coupled two pseudospin components of a Bose-Einstein condensate trapped in a quasi-one-dimensional harmonic potential, by using variational and directly numerical approach of binary mean-field Gross-Pitaevskii equations. The results show that, because of strong coupling of spin-orbit coupling (SOC), Rabi coupling, and atomic interaction, the collective dynamics of the system behave as complex characters. When the Rabi coupling is absent, the density profiles of the system preserve the Gauss type and the wave packets do harmonic oscillations. The amplitude of the collective oscillations increases with SOC. Furthermore, when the SOC strength increases, the dipole oscillations of the two pseudospin components undergo a transition from in-phase to out-of-phase oscillations. When the Rabi coupling present, there will exist a critical value of SOC strength (which depends on the Rabi coupling and atomic interaction). If the SOC strength is less than this critical value, the density profiles of the system can preserve the Gauss type and the wave packets do anharmonic (the frequency of dipole oscillations depends on SOC) oscillations synchronously (i.e., in-phase oscillations). However, if the SOC strength is larger than this critical value, the wave packets are dynamically fragmented and the stable dipole oscillations of the system can not exist. The collective dynamics of the system can be controlled by adjusting the atomic interaction, SOC, and Rabi-coupling strength.

  18. Dynamic susceptibility evidence of surface spin freezing in ultrafine NiFe2O4 nanoparticles.

    PubMed

    Tackett, Ronald J; Bhuiya, Abdul W; Botez, Cristian E

    2009-11-01

    We investigated the dynamic behavior of ultrafine NiFe2O4 nanoparticles (average size D = 3.5 nm) that exhibit anomalous low temperature magnetic properties such as low saturation magnetization and high-field irreversibility in both M(H) and ZFC-FC processes. Besides the expected blocking of the superspin, observed at T1 approximately 45 K, the system undergoes a magnetic transition at T2 approximately 6 K. For the latter, frequency- and temperature-resolved dynamic susceptibility data reveal characteristics that are unambiguously related to collective spin freezing: the relative variation (per frequency decade) of the in-phase susceptibility peak temperature is approximately 0.025, critical dynamics analysis yields an exponent znu = 9.6 and a zero-field freezing temperature T(F) = 5.8 K, and, in a magnetic field, T(F)(H) is excellently described by the de Almeida-Thouless line delta T(F) = 1 - T(F)(H)/T(F) alpha H(2/3). Moreover, out-of-phase susceptibility versus temperature datasets collected at different frequencies collapse on a universal dynamic scaling curve. All these observations indicate the existence of a spin-glass-like surface layer that surrounds the superparamagnetic core and undergoes a transition to a frozen state upon cooling below 5.8 K.

  19. ULTRAFAST ELECTRON SPIN DYNAMICS OF AS-GROWN Ga1-xMnxAs WITH APPROPRIATE Mn DOPING

    NASA Astrophysics Data System (ADS)

    Yue, Han

    2013-06-01

    The electron spin dynamics in the as-grown Ga1-xMnxAs films with appropriate Mn doping of x 2-5% is studied using time-resolved magneto-optical Kerr effect measurements. Due to the existence of Mn interstitials, the s-d exchange scattering is found to play an important role for the as-grown Ga1-xMnxAs, and compete with p-d exchange coupling to dominate the electron spin relaxation process. The contribution of electron-electron Coulomb scattering to the electron spin dynamics for the as-grown Ga1-x MnxAs appears to be as important as that of the annealed ones. Our findings are fundamentally important for better understanding the electron spin dynamics in Ga1-xMnxAs for its future spintronic applications.

  20. Multidimensional instability and dynamics of spin avalanches in crystals of nanomagnets.

    PubMed

    Jukimenko, O; Dion, C M; Marklund, M; Bychkov, V

    2014-11-21

    We obtain a fundamental instability of the magnetization-switching fronts in superparamagnetic and ferromagnetic materials such as crystals of nanomagnets, ferromagnetic nanowires, and systems of quantum dots with large spin. We develop the instability theory for both linear and nonlinear stages. By using numerical simulations we investigate the instability properties focusing on spin avalanches in crystals of nanomagnets. The instability distorts spontaneously the fronts and leads to a complex multidimensional front dynamics. We show that the instability has a universal physical nature, with a deep relationship to a wide variety of physical systems, such as the Darrieus-Landau instability of deflagration fronts in combustion, inertial confinement fusion, and thermonuclear supernovae, and the instability of doping fronts in organic semiconductors. PMID:25479521

  1. Attitude Dynamics of Spinning Solar Sail “IKAROS” Considering Thruster Plume

    NASA Astrophysics Data System (ADS)

    Mori, Osamu; Shirasawa, Yoji; Sawada, Hirotaka; Tsuda, Yuichi; Funase, Ryu; Saiki, Takanao; Yamamoto, Takayuki; Motooka, Norizumi; Jifuku, Ryo

    In this paper, the attitude dynamics of IKAROS, which is spinning solar sail, are presented. The first mode model of out-of-plane sail deformation (FMM) and multi-particle model (MPM) are introduced to analyze the oscillatory motion of the spinning solar sail. Three oscillation modes are derived from the FMM. They are caused by the nutation motion of the main body, as well as the nutation motion and the out-of-plane oscillation of the sail. The precise attitude motion after sail deployment and reorientation using thrusters is calculated using the MPM considering thruster plume. The IKAROS flight data of the nutation angular velocities of the main body after sail deployment or reorientation using thrusters are nearly equal to the analytical data found using the FMM and MPM.

  2. Implementation of Dynamically Corrected Gates on a Single Electron Spin in Diamond

    NASA Astrophysics Data System (ADS)

    Rong, Xing; Geng, Jianpei; Wang, Zixiang; Zhang, Qi; Ju, Chenyong; Shi, Fazhan; Duan, Chang-Kui; Du, Jiangfeng

    2014-02-01

    Precise control of an open quantum system is critical to quantum information processing but is challenging due to inevitable interactions between the quantum system and the environment. We demonstrated experimentally a type of dynamically corrected gates using only bounded-strength pulses on the nitrogen-vacancy centers in diamond. The infidelity of quantum gates caused by a nuclear-spin bath is reduced from being the second order to the sixth order of the noise-to-control-field ratio, which offers greater efficiency in reducing infidelity. The quantum gates have been protected to the limit essentially set by the spin-lattice relaxation time T1. Our work marks an important step towards fault-tolerant quantum computation in realistic systems.

  3. Spin dynamics and implications for superconductivity: Some problems with the d-wave scenario

    SciTech Connect

    Levin, K.; Zha, Y.; Radtke, R.J.; Si, Q.; Norman, M.R.; Schuttler, H.B.

    1993-09-01

    We review the spin dynamics of the normal state of the cuprates with special emphasis on neutron data in both the YBa{sub 2}Cu{sub 3}O{sub 7-{delta}} and La{sub 2-x}Sr{sub x}CuO{sub 4} systems. When realistic models of the Fermi surface shapes are incorporated, along with a moderate degree of spin fluctuations, we find good semi-quantiative agreement with experiment for both cuprates. Building on the success of this Fermi-liquid-based scheme, we explore the implications for d-wave pairing from a number of vantage points. We conclude that our present experimental and theoretical understanding is inadequate to confirm or refute the d-wave scenario.

  4. Multidimensional Instability and Dynamics of Spin Avalanches in Crystals of Nanomagnets

    NASA Astrophysics Data System (ADS)

    Jukimenko, O.; Dion, C. M.; Marklund, M.; Bychkov, V.

    2014-11-01

    We obtain a fundamental instability of the magnetization-switching fronts in superparamagnetic and ferromagnetic materials such as crystals of nanomagnets, ferromagnetic nanowires, and systems of quantum dots with large spin. We develop the instability theory for both linear and nonlinear stages. By using numerical simulations we investigate the instability properties focusing on spin avalanches in crystals of nanomagnets. The instability distorts spontaneously the fronts and leads to a complex multidimensional front dynamics. We show that the instability has a universal physical nature, with a deep relationship to a wide variety of physical systems, such as the Darrieus-Landau instability of deflagration fronts in combustion, inertial confinement fusion, and thermonuclear supernovae, and the instability of doping fronts in organic semiconductors.

  5. A Comparison Study of Magnetic Bearing Controllers for a Fully Suspended Dynamic Spin Rig

    NASA Technical Reports Server (NTRS)

    Choi, Benjamin; Johnson, Dexter; Morrison, Carlos; Mehmed, Oral; Huff, Dennis (Technical Monitor)

    2002-01-01

    NASA Glenn Research Center (GRC) has developed a fully suspended magnetic bearing system for the Dynamic Spin Rig (DSR) that is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust bearing and the associated control system were integrated into the DSR to provide noncontact magnetic suspension and mechanical excitation of the 35 lb vertical rotor with blades to induce turbomachinery blade vibration. A simple proportional-integral-derivative (PID) controller with a special feature for multidirectional radial excitation worked very well to both support and shake the shaft with blades. However, more advanced controllers were developed and successfully tested to determine the optimal controller in terms of sensor and processing noise reduction, smaller rotor orbits, and energy savings for the system. The test results of a variety of controllers we demonstrated up to the rig's maximum allowable speed of 10,000 rpm are shown.

  6. Breakdown of the field-induced superconductivity by dynamical spin reversal

    NASA Astrophysics Data System (ADS)

    Oshima, Yugo; Nojiri, Hiroyuki; Uji, Shinya; Brooks, James S.; Tokumoto, Takahisa; Cui, Heng-Bo; Kato, Reizo; Kobayashi, Akiko; Kobayashi, Hayao

    2012-07-01

    The quasi-two-dimensional molecular conductor λ-(BETS)2FeCl4, where BETS is bis(ethylenedithio)tetraselenafulvalene, shows a superconductivity in the high magnetic field environment. This is due to the compensation effect between the external field and the internal field created by the Fe3+ magnetic moment. Here, we report the simultaneous transport and electron spin resonance (ESR) measurements in the field-induced superconducting state down to 1.65 K. We find that the field-induced superconductivity is partially destroyed by ESR transitions, namely, by dynamical spin reversals of Fe3+. Moreover, it is found from our ESR results that the field-induced superconducting state is inhomogeneous, coexisting with the residual paramagnetic metal state.

  7. Multidimensional instability and dynamics of spin avalanches in crystals of nanomagnets.

    PubMed

    Jukimenko, O; Dion, C M; Marklund, M; Bychkov, V

    2014-11-21

    We obtain a fundamental instability of the magnetization-switching fronts in superparamagnetic and ferromagnetic materials such as crystals of nanomagnets, ferromagnetic nanowires, and systems of quantum dots with large spin. We develop the instability theory for both linear and nonlinear stages. By using numerical simulations we investigate the instability properties focusing on spin avalanches in crystals of nanomagnets. The instability distorts spontaneously the fronts and leads to a complex multidimensional front dynamics. We show that the instability has a universal physical nature, with a deep relationship to a wide variety of physical systems, such as the Darrieus-Landau instability of deflagration fronts in combustion, inertial confinement fusion, and thermonuclear supernovae, and the instability of doping fronts in organic semiconductors.

  8. Dynamical correlation effects on structure factor of spin-polarized two-dimensional electron gas

    SciTech Connect

    Singh, Gurvinder; Moudgil, R. K.; Kumar, Krishan; Garg, Vinayak

    2015-06-24

    We report a theoretical study on static density structure factor S(q) of a spin-polarized two-dimensional electron gas over a wide range of electron number density r{sub s}. The electron correlations are treated within the dynamical version of the self-consistent mean-field theory of Singwi, Tosi, Land, and Sjolander, the so-called qSTLS approach. The calculated S(q) exhibits almost perfect agreement with the quantum Monte Carlo simulation data at r{sub s}=1. However, the extent of agreement somewhat diminishes with increasing r{sub s}, particularly for q around 2k{sub F}. Seen in conjunction with the success of qSTLS theory in dealing with correlations in the unpolarized phase, our study suggests that the otherwise celebrated qSTLS theory is not that good in treating the like-spin correlations.

  9. Tracking the charge and spin dynamics of electronic excited states in inorganic complexes

    NASA Astrophysics Data System (ADS)

    Gaffney, Kelly

    2015-03-01

    Inorganic complexes have many advantageous properties for solar energy applications, including strong visible absorption and photocatalytic activity. Whether used as a photocatalyst or a photosensitizer, the lifetime of electronic excited states and the earth abundance of the molecular components represent a key property for solar energy applications. These dual needs have undermined the usefulness of many coordination compounds. Isoelectronic iron and ruthenium based complexes represent a clear example. Ru-polypyridal based molecules have been the workhorse of solar energy related research and dye sensitized solar cells for decades, but the replacement of low abundance Ru with Fe leads to million-fold reductions in metal to ligand charge transfer (MLCT) excited state lifetimes. Understanding the origin of this million-fold reduction in lifetime and how to control excited state relaxation in 3d-metal complexes motivates the work I will discuss. We have used the spin sensitivity of hard x-ray fluorescence spectroscopy and the intense femtosecond duration pulses generated by the LCLS x-ray laser to probe the spin dynamics in a series of electronically excited [Fe(CN)6-2N(2,2'-bipyridine)N]2 N - 4 complexes, with N = 1-3. These femtosecond resolution measurements demonstrate that modification of the solvent and ligand environment can lengthen the MLCT excited state lifetime by more than two orders of magnitude. They also verify the role of triplet ligand field excited states in the spin crossover dynamics from singlet to quintet spin configurations. Work supported by the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy.

  10. DYNAMICAL SPIN SUSCEPTIBILITY IN THE TD-LDA AND QSGW APPROXIMATIONS

    SciTech Connect

    SCHILFGAARDE, MARK VAN; KOTANI, TAKAO

    2012-10-15

    Abstract. This project was aimed at building the transverse dynamical spin susceptibility with the TD-LDA and the recently-developed Quasparticle Self-Consisent Approximations, which determines an optimum quasiparticle picture in a self-consistent manner within the GW approximation. Our main results were published into two papers, (J. Phys. Cond. Matt. 20, 95214 (2008), and Phys. Rev. B83, 060404(R) (2011). In the first paper we present spin wave dispersions for MnO, NiO, and -MnAs based on quasiparticle self-consistent GW approximation (QSGW). For MnO and NiO, QSGW results are in rather good agreement with experiments, in contrast to the LDA and LDA+U descriptions. For -MnAs, we find a collinear ferromagnetic ground state in QSGW, while this phase is unstable in the LDA. In the second, we apply TD-LDA to the CaFeAs2 the first attempt the first ab initio calculation of dynamical susceptibililty in a system with complex electronic structure Magnetic excitations in the striped phase of CaFe2As2 are studied as a function of local moment amplitude. We find a new kind of excitation: sharp resonances of Stoner-like (itinerant) excitations at energies comparable to the ´eel temperature, originating largely from a narrow band of Fe d states near the Fermi level, and coexisting with more conventional (localized) spin waves. Both kinds of excitations can show multiple branches, highlighting the inadequacy of a description based on a localized spin model.

  11. Optical studies of spin dynamics and hole transitions in ferromagnetic semiconductor (gallium,manganese)arsenic

    NASA Astrophysics Data System (ADS)

    Wang, Daimian

    The ferromagnetic semiconductor (Ga,Mn)As has been a focus of much research prompted by its potential applications in semiconductor spintronics. In this thesis, studies of the defect configuration and spin dynamics in this material are reported. The technique of resonant Raman scattering was used to study the defect configuration. Insulating nano-islands consisting of substitutional Mn Ga acceptors and interstitial MnI donors were observed in ferromagnetic (Ga,Mn)As from resonant Raman spectra. As indicated by a sharp Raman transition from the 1S3/2-2 S3/2 hole levels at 703 cm-1, holes bound to MnGa acceptors inside the islands are partially isolated from the outside ferromagnetic environment. The MnGa ions inside the islands can interact with the ferromagnetic environment through bound excitons, as suggested by the presence of magnon-related side peaks. The radius of the nano-islands is inferred to be 5-10 nm. The islands disappear after annealing due to the removal of the MnI ions. Furthermore, the technique of pump-probe magneto-optical Kerr spectroscopy was used to study the spin dynamics in (Ga,Mn)As. Coherent oscillations associated with magnetization precessions were observed. Using a comprehensive theoretical description of the processes by which light couples to the magnetization, the anisotropy and spin stiffness constants were gained from the experimental data. Results reveal a relatively large negative contribution to the energy due to surface anisotropy leading to excitations that are a mixture of bulk waves and surface modes. The dependence of the spin wave oscillations on magnetic field direction and temperature is also discussed. Finally, the pump-probe technique was used to study interlayer coupling in (Ga,Mn)As-based superlattices. A coupled spin precession mode was observed in two layers of (Ga,Mn)As seperated by two-monolayers of AlAs. The spin wave spectra on superlattices with GaAs as spacer layers imply that Mn ions diffuse from (Ga,Mn)As to

  12. Mixed Ising system designed with integer and half-integer spins: dynamic behaviors under oscillating magnetic field

    NASA Astrophysics Data System (ADS)

    Ertaş, Mehmet

    2016-06-01

    By using the simplified effective-field theory based on Glauber-type stochastic dynamics, namely the dynamic simplified effective-field theory, the dynamic phase diagrams of a two-dimensional mixed spin-1 and spin-3/2 Blume-Capel model are studied in an oscillating external magnetic field. The dynamic equations are derived for two interpenetrating square lattices. The time variations of average magnetizations and the temperature dependence of the dynamic magnetizations are examined, and the dynamic phase diagrams are presented in the two different planes. The dynamic phase diagrams illustrate several ordered phases, the coexistence phase region and critical points as well as a re-entrant behavior depending on the interaction parameters. Finally, the discussion and comparison of the dynamic phase diagrams are given briefly.

  13. Magnetic friction of a nanometer-sized tip scanning a magnetic surface: Dynamics of a classical spin system with direct exchange and dipolar interactions between the spins

    NASA Astrophysics Data System (ADS)

    Fusco, C.; Wolf, D. E.; Nowak, U.

    2008-05-01

    We theoretically study the occurrence of magnetic friction of a nanometer-sized tip scanning a magnetic surface by studying the dynamics of a model of classical spins interacting through dipolar and exchange interactions, neglecting thermal effects. We find that for small scanning velocities, the friction force linearly scales with the velocity, with a slope proportional to the phenomenological damping parameter of the Landau-Lifshitz-Gilbert equation. At higher velocities, the friction vs velocity relationship becomes rather complex with the presence of a maximum that is explained by the excitations of spin-wave resonances in the sample.

  14. Dynamics of intramolecular spin exchange interaction of a nitronyl nitroxide diradical in solution and on surfaces

    NASA Astrophysics Data System (ADS)

    Lloveras, V.; Badetti, E.; Veciana, J.; Vidal-Gancedo, J.

    2016-02-01

    In this paper we report the study of the dynamics of a thermally modulated intramolecular spin exchange interaction of a novel diradical nitronyl nitroxide-substituted disulfide in solution and when it is grafted on a gold surface. The structure of this diradical was designed to have flexible chains leading to intramolecular collisions and hence spin exchange interaction, and with an appropriate binding group to be grafted on the gold surface to study its behavior on the surface. In solution, this diradical shows a strong spin exchange interaction between both radicals which is modulated by temperature, but also gold nanoparticles (AuNPs) functionalized with this diradical permit investigation of such a phenomenon in surface-grafted radicals. The spin-labelled AuNP synthesis was optimized to obtain high coverage of spin labels to lead to high spin exchange interaction. The obtained AuNPs were studied by Electron Paramagnetic Resonance (EPR), UV-Vis, and IR spectroscopies, HR-TEM microscopy, Cyclic Voltammetry (CV), Energy Dispersive X-ray analysis (EDX) and Thermogravimetric Analysis (TGA). This inorganic-organic hybrid material also showed dipolar interactions between its radicals which were confirmed by the appearance in the EPR spectra of an |Δms| = 2 transition at half-field. This signal gives direct evidence of the presence of a high-spin state and permitted us to study the nature of the magnetic coupling between the spins which was found to be antiferromagnetic. Self-Assembled Monolayers (SAMs) of these radicals on the Au (111) substrate were also prepared and studied by contact angle, X-Ray Photoelectron Spectroscopy (XPS), Time-of-Flight Secondary Ion Mass Spectrometry (ToF-SIMS), Cyclic Voltammetry and EPR. The magnetic as well as the electrochemical properties of the hybrid surfaces were studied and compared with the properties of this diradical in solution. Analogies between the properties of AuNPs with high coverage of radicals and those of SAM were

  15. A theoretical analysis of the spin dynamics of magnetic adatoms traced by time-resolved scanning tunneling spectroscopy

    NASA Astrophysics Data System (ADS)

    Schüler, M.; Pavlyukh, Y.; Berakdar, J.

    2012-04-01

    Inelastic scanning tunneling microscopy (STM) has recently been shown (Loth et al 2010 Science 329 1628) to be extendable to access the nanosecond, spin-resolved dynamics of magnetic adatoms and molecules. Here we analyze this novel tool theoretically by considering the time-resolved spin dynamics of a single adsorbed Fe atom excited by a tunneling current pulse from a spin-polarized STM tip. The adatom spin configuration can be controlled and probed by applying voltage pulses between the substrate and the spin-polarized STM tip. We demonstrate how, in a pump-probe manner, the relaxation dynamics of the sample spin is manifested in the spin-dependent tunneling current. Our model calculations are based on the scattering theory in a wave-packet formulation. The scheme is non-perturbative and, hence, is valid for all voltages. The numerical results for the tunneling probability and the conductance are contrasted with the predictions of simple analytical models and compared with experiments.

  16. Optimal pulse spacing for dynamical decoupling in the presence of a purely dephasing spin bath

    SciTech Connect

    Ajoy, Ashok; Alvarez, Gonzalo A.; Suter, Dieter

    2011-03-15

    Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are {sup 13}C nuclear spins and the environment consists of a {sup 1}H nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.

  17. Multi-triplet bound states and finite-temperature dynamics in highly frustrated quantum spin ladders

    NASA Astrophysics Data System (ADS)

    Honecker, Andreas; Mila, Frédéric; Normand, B.

    2016-09-01

    Low-dimensional quantum magnets at finite temperatures present a complex interplay of quantum and thermal fluctuation effects in a restricted phase space. While some information about dynamical response functions is available from theoretical studies of the one-triplet dispersion in unfrustrated chains and ladders, little is known about the finite-temperature dynamics of frustrated systems. Experimentally, inelastic neutron scattering studies of the highly frustrated two-dimensional material SrCu2(BO3)2 show an almost complete destruction of the one-triplet excitation band at a temperature only 1/3 of its gap energy, accompanied by strong scattering intensities for apparent multi-triplet excitations. We investigate these questions in the frustrated spin ladder and present numerical results from exact diagonalization for the dynamical structure factor as a function of temperature. We find anomalously rapid transfer of spectral weight out of the one-triplet band and into both broad and sharp spectral features at a wide range of energies, including below the zero-temperature gap of this excitation. These features are multi-triplet bound states, which develop particularly strongly near the quantum phase transition, fall to particularly low energies there, and persist all the way to infinite temperature. Our results offer valuable insight into the physics of finite-temperature spectral functions in SrCu2(BO3)2 and many other highly frustrated spin systems.

  18. All electrical manipulation of magnetization dynamics in a ferromagnet by antiferromagnets with anisotropic spin Hall effects.

    SciTech Connect

    Zhang, Wei; Jungfleisch, Matthias B.; Freimuth, Frank; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Mokrousov, Yuri; Hoffmann, Axel

    2015-10-06

    We investigate spin-orbit torques of metallic CuAu-I-type antiferromagnets using spin-torque ferromagnetic resonance tuned by a dc-bias current. The observed spin torques predominantly arise from diffusive transport of spin current generated by the spin Hall effect. We find a growth-orientation dependence of the spin torques by studying epitaxial samples, which may be correlated to the anisotropy of the spin Hall effect. The observed anisotropy is consistent with first-principles calculations on the intrinsic spin Hall effect. Our work suggests large tunable spin-orbit effects in magnetically-ordered materials.

  19. Instrumentation for solid-state dynamic nuclear polarization with magic angle spinning NMR.

    PubMed

    Rosay, Melanie; Blank, Monica; Engelke, Frank

    2016-03-01

    Advances in dynamic nuclear polarization (DNP) instrumentation and methodology have been key factors in the recent growth of solid-state DNP NMR applications. We review the current state of the art of solid-state DNP NMR instrumentation primarily based on available commercial platforms. We start with a general system overview, including options for microwave sources and DNP NMR probes, and then focus on specific developments for DNP at 100K with magic angle spinning (MAS). Gyrotron microwave sources, passive components to transmit microwaves, the DNP MAS probe, a cooling device for low-temperature MAS, and sample preparation procedures including radicals for DNP are considered. PMID:26920834

  20. Calibration of the spin-scan ozone imager aboard the dynamics Explorer 1 satellite

    NASA Technical Reports Server (NTRS)

    Bressette, Walter E.; Keating, Gerald M.; Young, David F.

    1987-01-01

    The calibration technique, which contains the calibrated backscattered radiance values necessary for performing the calibrations, is presented. The calibration constants for September to October 1981 to determine total columnar ozone from the Spin-Scan Ozone Imager (SOI), which is a part of the auroral imaging instrumentation aboard the Dynamics Explorer 1 Satellite, are provided. The precision of the SOI-derived total columnar ozone is estimated to be better than 2.4 percent. Linear regression analysis was used to calculate correlation coefficients between total columnar ozone obtained from Dobson ground stations and SOI which indicate that the SOI total columnar ozone determination is equally accurate for clear or cloudy weather conditions.

  1. Quench dynamics of 1D spin-imbalanced Fermi-Hubbard model

    NASA Astrophysics Data System (ADS)

    Yin, Xiao; Radzihovsky, Leo

    We study a non-equilibrium dynamics of a 1D spin-imbalanced Fermi-Hubbard model following a quantum quench of on-site interaction, using bosonization and exact analysis. By focusing on the evolution of singlet-, triplet-, density and magnetization correlation functions, we find that the evolution and the final state display a strong dependence on the initial state. Thus, we demonstrate that such quantum quench may be used as a new approach to identify and probe the 1D gapless analogue of the elusive FFLO state. Supported by NSF through DMR-1001240 and by Simons Investigator award from Simons.

  2. Spin Dynamics in Two-Dimensional Arrays of Quantum Dots with Local Ordering of Nanoclusters

    SciTech Connect

    Zinovieva, A. F.; Dvurechenskii, A. V.; Stepina, N. P.; Nikiforov, A. I.; Lyubin, A. S.; Sobolev, N.; Carmo, M. C.

    2011-12-23

    Electron paramagnetic resonance (EPR) is used to probe the spin dynamics in two-dimensional (2D) quantum dot (QD) arrays with local ordering of nanoclusters. A careful examination of EPR line shape, width and g-factor values allow us to attribute this signal to the electrons localized in the strain-induced potential wells in Si in the vicinity of the Ge dots. The strong orientation dependence of EPR line width is defined by changing localization degree of electrons at different magnetic field directions. The theoretical approximation of orientation dependence of EPR line width allows estimating the effective radius of electron localization, as {approx}80 nm.

  3. Dynamics of quantized vortices in Bose-Einstein condensates with laser-induced spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    Kasamatsu, Kenichi

    2015-12-01

    We study vortex dynamics in trapped two-component Bose-Einstein condensates with a laser-induced spin-orbit coupling using the numerical analysis of the Gross-Pitaevskii equation. The spin-orbit coupling leads to three distinct ground-state phases, which depend on some experimentally controllable parameters. When a vortex is put in one or both of the two-component condensates, the vortex dynamics exhibits very different behaviors in each phase, which can be observed in experiments. These dynamical behaviors can be understood by clarifying the stable vortex structure realized in each phase.

  4. Spin-dependent studies of the dynamics of He(2 3S) atom deexcitation at surfaces

    NASA Astrophysics Data System (ADS)

    Dunning, F. B.; Nordlander, P.

    1995-06-01

    Electron spin labelling techniques provide a powerful technique with which to probe the dynamics of He(2 3S) atom deexcitation at surfaces. Studies with a clean Cu(100) surface reveal that deexcitation occurs exclusively through resonance ionization followed by Auger neutralization and that the electrons involved in Auger neutralization are correlated in spin. Model calculations suggest that this can be explained by considering the local perturbation in the surface electronic structure induced by the presence of the (polarized) He + ion. The calculated induced densities of states are spin dependent and exhibit sharp Kondo-like resonances near the Fermi level. Measurements at an adsorbed Xe film are also described and suggest that electron ejection results both from direct Auger deexcitation (surface Penning ionization) and from resonance ionization of incident atoms, the resulting ions being neutralized through an interaction that involves neighboring Xe atoms in the film. The Xe film data provide an unusual example of a surface at which resonance ionization and Auger deexcitation occur in parallel with comparable rates.

  5. Phenomenological Theory of Spin-Glasses ---Static Non-Linear and Dynamical Linear Susceptibilities---

    NASA Astrophysics Data System (ADS)

    Honda, K.; Nakano, H.

    1981-01-01

    By talking into account a symmetry consideration in the theory proposed by the present authors (Prog. Theor. Phys. 65 (1981), 83), the expression for free energy of spin-glass is obtained as a function of the respective parameters g and m for spin-glass and ferromagnetic phases and of what was named the internal field parameter θ. It is found that the non-linear susceptibility χ2 diverges to minus infinity at the transition temperature T_g between the spin-glass and paramagnetic phases in proportion to |T-T_g|-1. On the basis of a conventional theory, the kinetic equation for g, m and θ are constructed to calculate the dynamical susceptibility χ(ω). A collective mode exhibiting the critical slowing down at T_g is found from the poles of χ(ω). The imaginary part of χ(ω) divided by the frequency ω diverges to infinity in the vanishing limit of ω with critical exponents different adjacently below and above T_g.

  6. Magnetic Dynamics of Single-Domain Planar Spin-Transfer Devices

    NASA Astrophysics Data System (ADS)

    Bazaliy, Ya. B.

    2008-03-01

    We study spin-transfer devices with dynamic magnets characterized by large easy-plane anisotropy. This situation is standard for planar devices where it arises due to the shape anisotropy. Dominating easy-plane anisotropy keeps the motion of the magnetic moment close to the easy plane, with small out-of-plane deviations. As a result, it is possible to approximately describe magnetization vector by the in-plane angle and derive an effective one dimensional equation for that angle in the absence [1] and in the presence [2] of spin-transfer torques. Effective description maps a spin-transfer device problem onto a problem of an ``effective particle'' moving in external potential with variable friction coefficient. The advantage of such a description is that the motion of the effective particle can be qualitatively understood by applying the usual energy conservation and dissipation arguments. We show how the effective description produces analytic results for current induced precession states [3] and predicts unconventional ``stabilization by repulsion'' of static states [2]. // [1] C. J. Garcia-Cervera, Weinan E, J. Appl. Phys. 90, 370 (2001). [2] Ya. B. Bazaliy, Phys. Rev. B 76, 140402(R) (2007). [3] Ya. B. Bazaliy, arXiv:0705.0508, to be published in Appl. Phys. Lett. (2007).

  7. Molecular dynamics in rod-like liquid crystals probed by muon spin resonance spectroscopy.

    PubMed

    McKenzie, Iain; Scheuermann, Robert; Sedlak, Kamil; Stoykov, Alexey

    2011-08-01

    Muoniated spin probes were produced by the addition of muonium (Mu) to two rod-like liquid crystals: N-(4-methoxybenzylidene)-4'-n-butylaniline (MBBA) and cholesteryl nonanoate (CN). Avoided level crossing muon spin resonance spectroscopy was used to characterize the muoniated spin probes and to probe dynamics at the molecular level. In MBBA Mu adds predominantly to the carbon of the bridging imine group and the muon and methylene proton hyperfine coupling constants (hfccs) of the resulting radical shift in the nematic phase due to the dipolar hyperfine coupling, the ordering of the molecules along the applied magnetic field and fluctuations about the local director. The amplitude of these fluctuations in in the nematic phase of MBBA is determined from the temperature dependence of the methylene proton hfcc. Mu adds to the double bond of the steroidal ring system of CN and the temperature dependence of the Δ(1) line width provides information about the amplitude of the fluctuations about the local director in the chiral nematic phase and the slow isotropic reorientation in the isotropic phase.

  8. Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR

    SciTech Connect

    Seung-Ho-Baek

    2004-12-19

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T{sub l}) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T{sub l} probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.

  9. Cyclotron dynamics of a Kondo singlet in a spin-orbit-coupled alkaline-earth-metal atomic gas

    NASA Astrophysics Data System (ADS)

    Jiang, Bo-Nan; Lv, Hao; Wang, Wen-Li; Du, Juan; Qian, Jun; Wang, Yu-Zhu

    2014-11-01

    We propose a scheme to investigate the interplay between the Kondo-exchange interaction and the quantum spin Hall effect with ultracold fermionic alkaline-earth-metal atoms trapped in two-dimensional optical lattices using ultracold collision and laser-assisted tunneling. In the strong Kondo-coupling regime, although the loop trajectory of the mobile atom disappears, collective dynamics of an atom pair in two clock states can exhibit an unexpected spin-dependent cyclotron orbit in a plaquette, realizing the quantum spin Hall effect of the Kondo singlet. We demonstrate that the collective cyclotron dynamics of the spin-zero Kondo singlet is governed by an effective Harper-Hofstadter model in addition to second-order diagonal tunneling.

  10. Polynomially scaling spin dynamics II: Further state-space compression using Krylov subspace techniques and zero track elimination

    NASA Astrophysics Data System (ADS)

    Kuprov, Ilya

    2008-11-01

    We extend the recently proposed state-space restriction (SSR) technique for quantum spin dynamics simulations [Kuprov et al., J. Magn. Reson. 189 (2007) 241-250] to include on-the-fly detection and elimination of unpopulated dimensions from the system density matrix. Further improvements in spin dynamics simulation speed, frequently by several orders of magnitude, are demonstrated. The proposed zero track elimination (ZTE) procedure is computationally inexpensive, reversible, numerically stable and easy to add to any existing simulation code. We demonstrate that it belongs to the same family of Krylov subspace techniques as the well-known Lanczos basis pruning procedure. The combined SSR + ZTE algorithm is recommended for simulations of NMR, EPR and Spin Chemistry experiments on systems containing between 10 and 10 4 coupled spins.

  11. Polynomially scaling spin dynamics II: further state-space compression using Krylov subspace techniques and zero track elimination.

    PubMed

    Kuprov, Ilya

    2008-11-01

    We extend the recently proposed state-space restriction (SSR) technique for quantum spin dynamics simulations [Kuprov et al., J. Magn. Reson. 189 (2007) 241-250] to include on-the-fly detection and elimination of unpopulated dimensions from the system density matrix. Further improvements in spin dynamics simulation speed, frequently by several orders of magnitude, are demonstrated. The proposed zero track elimination (ZTE) procedure is computationally inexpensive, reversible, numerically stable and easy to add to any existing simulation code. We demonstrate that it belongs to the same family of Krylov subspace techniques as the well-known Lanczos basis pruning procedure. The combined SSR+ZTE algorithm is recommended for simulations of NMR, EPR and Spin Chemistry experiments on systems containing between 10 and 10(4) coupled spins.

  12. Vortex Dynamics in a Spin-Orbit-Coupled Bose-Einstein Condensate

    NASA Astrophysics Data System (ADS)

    Fetter, Alexander L.

    2015-07-01

    Vortices in a one-component dilute atomic ultracold Bose-Einstein condensate (BEC) usually arise as a response to externally driven rotation. Apart from a few special situations, these vortices are singly quantized with unit circulation (Fetter, Rev Mod Phys 81, 647-691, 2009). Recently, the NIST group has constructed a two-component BEC with a spin-orbit-coupled Hamiltonian involving Pauli matrices (Spielman, Phys Rev A 79, 063613, 2009; Y.-J. Lin et al., Nature 462, 628-632, 2009; Y.-J. Lin et al., Nature 471, 83-87, 2011), and I here study the dynamics of a two-component vortex in such a spin-orbit-coupled condensate. These spin-orbit-coupled BECs use an applied magnetic field to split the hyperfine levels. Hence, they rely on a focused laser beam to trap the atoms. In addition, two Raman laser beams create an effective (or synthetic) gauge potential. The resulting spin-orbit Hamiltonian is discussed in some detail. The various laser beams are fixed in the laboratory, so that it is not feasible to nucleate a vortex by an applied rotation that would need to rotate all the laser beams and the magnetic field. In a one-component BEC, a vortex can also be created by a thermal quench, starting from the normal state and suddenly cooling deep into the condensed state (Freilich et al., Science 329, 1182-1185, 2010). I propose that a similar method would work for a vortex in a spin-orbit-coupled BEC. Such a vortex has two components, and each has its own circulation quantum number (typically ). If both components have the same circulation, I find that the composite vortex should execute uniform precession, like that observed in a single-component BEC (Freilich et al., Science 329, 1182-1185, 2010). In contrast, if one component has unit circulation and the other has zero circulation, then some fraction of the dynamical vortex trajectories should eventually leave the condensate, providing clear experimental evidence for this unusual vortex structure. In the context of

  13. Nuclear depolarization and absolute sensitivity in magic-angle spinning cross effect dynamic nuclear polarization.

    PubMed

    Mentink-Vigier, Frédéric; Paul, Subhradip; Lee, Daniel; Feintuch, Akiva; Hediger, Sabine; Vega, Shimon; De Paëpe, Gaël

    2015-09-14

    Over the last two decades solid state Nuclear Magnetic Resonance has witnessed a breakthrough in increasing the nuclear polarization, and thus experimental sensitivity, with the advent of Magic Angle Spinning Dynamic Nuclear Polarization (MAS-DNP). To enhance the nuclear polarization of protons, exogenous nitroxide biradicals such as TOTAPOL or AMUPOL are routinely used. Their efficiency is usually assessed as the ratio between the NMR signal intensity in the presence and the absence of microwave irradiation εon/off. While TOTAPOL delivers an enhancement εon/off of about 60 on a model sample, the more recent AMUPOL is more efficient: >200 at 100 K. Such a comparison is valid as long as the signal measured in the absence of microwaves is merely the Boltzmann polarization and is not affected by the spinning of the sample. However, recent MAS-DNP studies at 25 K by Thurber and Tycko (2014) have demonstrated that the presence of nitroxide biradicals combined with sample spinning can lead to a depolarized nuclear state, below the Boltzmann polarization. In this work we demonstrate that TOTAPOL and AMUPOL both lead to observable depolarization at ≈110 K, and that the magnitude of this depolarization is radical dependent. Compared to the static sample, TOTAPOL and AMUPOL lead, respectively, to nuclear polarization losses of up to 20% and 60% at a 10 kHz MAS frequency, while Trityl OX63 does not depolarize at all. This experimental work is analyzed using a theoretical model that explains how the depolarization process works under MAS and gives new insights into the DNP mechanism and into the spin parameters, which are relevant for the efficiency of a biradical. In light of these results, the outstanding performance of AMUPOL must be revised and we propose a new method to assess the polarization gain for future radicals.

  14. Dynamical passage to approximate equilibrium shapes for spinning, gravitating rubble asteroids

    NASA Astrophysics Data System (ADS)

    Sharma, Ishan; Jenkins, James T.; Burns, Joseph A.

    2009-03-01

    Many asteroids are thought to be particle aggregates held together principally by self-gravity. Here we study — for static and dynamical situations — the equilibrium shapes of spinning asteroids that are permitted for rubble piles. As in the case of spinning fluid masses, not all shapes are compatible with a granular rheology. We take the asteroid to always be an ellipsoid with an interior modeled as a rigid-plastic, cohesion-less material with a Drucker-Prager yield criterion. Using an approximate volume-averaged procedure, based on the classical method of moments, we investigate the dynamical process by which such objects may achieve equilibrium. We first collapse our dynamical approach to its statical limit to derive regions in spin-shape parameter space that allow equilibrium solutions to exist. At present, only a graphical illustration of these solutions for a prolate ellipsoid following the Drucker-Prager failure law is available [Sharma, I., Jenkins, J.T., Burns, J.A., 2005a. Bull. Am. Astron. Soc. 37, 643; Sharma, I., Jenkins, J.T., Burns, J.A., 2005b. Equilibrium shapes of ellipsoidal soil asteroids. In: García-Rojo, R., Hermann, H.J., McNamara, S. (Eds.), Proceedings of the 5th International Conference on Micromechanics of Granular Media, vol. 1. A.A. Balkema, UK; Holsapple, K.A., 2007. Icarus 187, 500-509]. Here, we obtain the equilibrium landscapes for general triaxial ellipsoids, as well as provide the requisite governing formulae. In addition, we demonstrate that it may be possible to better interpret the results of Richardson et al. [Richardson, D.C., Elankumaran, P., Sanderson, R.E., 2005. Icarus 173, 349-361] within the context of a Drucker-Prager material. The graphical result for prolate ellipsoids in the static limit is the same as those of Holsapple [Holsapple, K.A., 2007. Icarus 187, 500-509] because, when worked out, his final equations will match ours. This is because, though the formalisms to reach these expressions differ, in statics

  15. The ˜AD 1250 effusive eruption of El Metate shield volcano (Michoacán, Mexico): magma source, crustal storage, eruptive dynamics, and lava rheology

    NASA Astrophysics Data System (ADS)

    Chevrel, Magdalena Oryaëlle; Guilbaud, Marie-Noëlle; Siebe, Claus

    2016-04-01

    Medium-sized volcanoes, also known as Mexican shields due to their andesitic composition and slightly higher slope angles in comparison to Icelandic shields, occur across the Trans-Mexican Volcanic Belt and represent nearly one third of all volcanic edifices in the Michoacán-Guanajuato Volcanic Field (MGVF). Many questions about their origin and eruptive dynamics remain unanswered. Here, we focus on El Metate, the youngest (˜AD 1250) monogenetic shield volcano of the MGVF and the most voluminous (˜9.2 km3 dense rock equivalent) Holocene eruption in Mexico. Its eruptive history was reconstructed through detailed mapping, geochemical analysis (major and trace elements, Sr-Nd-Pb isotopic data), and rheological study of its thick andesitic flows. Early and late flow units have distinct morphologies, chemical and mineralogical compositions, and isotopic signatures which show that these lavas were fed by two separate magma batches that originated from a heterogeneous mantle source and followed distinct differentiation paths during their ascent. Thermobarometry calculations constraining the conditions of crystallization indicate a temporary storage of the last erupted magma batch at a depth of ˜7-10 km. Lava rheology was estimated using petrographic characteristics, geochemical data, and flow dimensions. The magma viscosity increased from 102-103 Pa s prior to eruption through 106-108 Pa s during ascent, to 109-1011 Pa s during lava emplacement. Though magma viscosity was quite high, the eruption was purely effusive. The explosive eruption of such a large magma volume was probably avoided due to efficient open system degassing (outgassing) of the magma as it ascended through the uppermost crust and erupted at the surface.

  16. Corium shield

    DOEpatents

    McDonald, Douglas B.; Buchholz, Carol E.

    1994-01-01

    A shield for restricting molten corium from flowing into a water sump disposed in a floor of a containment vessel includes upper and lower walls which extend vertically upwardly and downwardly from the floor for laterally bounding the sump. The upper wall includes a plurality of laterally spaced apart flow channels extending horizontally therethrough, with each channel having a bottom disposed coextensively with the floor for channeling water therefrom into the sump. Each channel has a height and a length predeterminedly selected for allowing heat from the molten corium to dissipate through the upper and lower walls as it flows therethrough for solidifying the molten corium therein to prevent accumulation thereof in the sump.

  17. Chiral shielding

    SciTech Connect

    Babukhadia, L.; Berdnikov, Ya. A.; Ivanov, A. N.; Scadron, M. D.

    2000-08-01

    We demonstrate how a chiral soft pion theorem (SPT) shields the scalar meson ground-state isoscalar {sigma}(600-700) and isospinor {kappa}(800-900) from detection in a{sub 1}{yields}{pi}({pi}{pi}){sub swave}, {gamma}{gamma}{yields}2{pi}{sup 0}, {pi}{sup -}p{yields}{pi}{sup -}{pi}{sup +}n and K{sup -}p{yields}K{sup -}{pi}{sup +}n processes. While pseudoscalar meson PVV transitions are known to be determined by (only) quark loop diagrams, the above SPT also constrains scalar meson SVV transitions to be governed (only) by meson loop diagrams. We apply this latter SVV theorem to a{sub 0}{yields}{gamma}{gamma} and f{sub 0}{yields}{gamma}{gamma} decays. (c) 2000 The American Physical Society.

  18. Application of a system modification technique to dynamic tuning of a spinning rotor blade

    NASA Technical Reports Server (NTRS)

    Spain, C. V.

    1987-01-01

    An important consideration in the development of modern helicopters is the vibratory response of the main rotor blade. One way to minimize vibration levels is to ensure that natural frequencies of the spinning main rotor blade are well removed from integer multiples of the rotor speed. A technique for dynamically tuning a finite-element model of a rotor blade to accomplish that end is demonstrated. A brief overview is given of the general purpose finite element system known as Engineering Analysis Language (EAL) which was used in this work. A description of the EAL System Modification (SM) processor is then given along with an explanation of special algorithms developed to be used in conjunction with SM. Finally, this technique is demonstrated by dynamically tuning a model of an advanced composite rotor blade.

  19. Dynamic structure factor of the spin-1/2 XXZ chain in a transverse field

    NASA Astrophysics Data System (ADS)

    Bruognolo, Benedikt; Weichselbaum, Andreas; von Delft, Jan; Garst, Markus

    2016-08-01

    The spin-1/2 XXZ chain with easy-plane anisotropy in a transverse field describes well the thermodynamic properties of the material Cs2CoCl4 in a wide range of temperatures and fields including the region close to the spin-flop Ising quantum phase transition. For a comparison with prospective inelastic neutron scattering experiments on this compound, we present results of an extensive numerical study of its dynamic structure factor Sα β(k ,ω ) using matrix-product-state (MPS) techniques. Close to criticality, the dynamic part of the correlator Sx x longitudinal to the applied field is incoherent and possesses a small total weight as the ground state is already close to saturation. The transverse correlator Sz z, on the other hand, is dominated by a coherent single-particle excitation with additional spectral weight at higher energies that we tentatively attribute to a repulsively bound pair of particles. With increasing temperature, the latter quickly fades and spectral weight instead accumulates close to zero wave vector just above the single-particle energy. On a technical level, we compare the numerical efficiency of real-time evolution to an MPS-based Chebyshev expansion in the present context, finding that both methods yield results of similar quality at comparable numerical costs.

  20. Dynamic magnetism of an iron(II)-chlorido spin chain and its hexametallic segment.

    PubMed

    Qin, Lei; Zhang, Zhong; Zheng, Zhiping; Speldrich, Manfred; Kögerler, Paul; Xue, Wei; Wang, Bao-Ying; Chen, Xiao-Ming; Zheng, Yan-Zhen

    2015-01-21

    An air-stable iron(ii) chain compound [Fe(phen)(Cl)2]n (, phen = 1,10-phenanthroline) was prepared and exhibits intrachain ferromagnetic interactions as well as competing interchain antiferromagnetic interactions that are mediated by π-π stacking of the phen ligands, resulting in metamagnetic behaviour. The interchain interactions can be altered by changing the external magnetic field, and disparate magnetic dynamics was thus observed from zero to the critical field of 1500 Oe. Zero-field cooled (ZFC) and field-cooled (FC) magnetization and heat capacity measurements indicate that long-range antiferromagnetic ordering occurs at lower fields, and this ordering disappears when the external field is larger than 1500 Oe. The low-frequency ac susceptibility data are consistent with the exponential increase of the temperature-dependent dc data, indicating a Glauber-type dynamics under the field of 1500 Oe. Thus, is considered as a metamagnetic single-chain magnet. For further analysis, a discrete hexametallic segment of the chain, [Fe6(phen)6(Cl)12] (), was also isolated and was shown to possess a high-spin ground state and display slow magnetic relaxations like single-molecule magnets. Magnetic analysis using CONDON suggests weak ferromagnetic interactions between the metal centres. The polymeric compound can be viewed as being constructed using the hexametallic unit which is of a low energy barrier, suggesting the significance of intrachain ferromagnetic interactions in enhancing the spin-reversal energy barrier of the short chains. PMID:25428779

  1. Nonlinear dynamics of a strongly driven single spin solid state qubit

    NASA Astrophysics Data System (ADS)

    Coppersmith, S. N.; Jullien, Thibaut; Scarlino, P.; Kawakami, E.; Ward, D. R.; Savage, D. E.; Lagally, M. G.; Friesen, Mark; Eriksson, M. A.; Vandersypen, L. M. K.

    This talk will discuss how dynamical systems theory can yield new insight into some exotic behavior found in experiments on strongly driven quantum spins in silicon/silicon-germanium heterostructures. Spin resonance experiments were performed by using ac voltages to drive an electron wavefunction in a strong magnetic field gradient. Nontrivial dependence of the resonance frequency on applied power, including the observation of multiple resonant frequencies at one power, are shown to be consistent with frequency-dependent attenuation in the high-frequency lines. The method of analysis is very similar to that presented in the course on nonlinear dynamics that Leo Kadanoff developed at the University of Chicago in the early 1990's. This work was supported in part by ARO (W911NF-12-0607). Development and maintenance of the growth facilities used for fabricating samples is supported by DOE (DE-FG02-03ER46028). This research utilized NSF-supported shared facilities at UW-Madison.

  2. Dynamical scalability and control of totally connected spin networks across quantum phase transitions

    NASA Astrophysics Data System (ADS)

    Acevedo, Óscar L.; Quiroga, Luis; Rodríguez, Ferney J.; Johnson, Neil F.

    2014-03-01

    Dynamical quantum phase crossings of spin networks have recently received increased attention thanks to their relation to adiabatic quantum computing, and their feasible realizations using ultra-cold atomic and molecular systems with a highly tunable degree of connectivity. Dynamical scaling of spatially distributed systems like Ising models have been widely studied, and successfully related to well-known theories like the Kibble-Zurek mechanism. The case of totally connected networks such as the Dicke Model and Lipkin-Meshkov-Glick Model, however, is known to exhibit a breakdown of these frameworks. Our analysis overcomes the lack of spatial correlation structure by developing a general approach which (i) is valid regardless the connectivity of the system, (ii) goes beyond critical exponents, and (iii) provides a time-resolved picture of dynamical scaling. By treating these models as a method for macroscopic quantum control of their subsystems, we have found microscopic signatures of the dynamical scaling as well as instances of dynamical enhancement of distinctive quantum properties such as entanglement and coherence. Our results yield novel prescriptions for the fields of quantum simulations and quantum control, and deepen our fundamental understanding of phase transitions.

  3. GCFR plenum shield design: exit shield experiment

    SciTech Connect

    Muckenthaler, F.J.; Hull, J.L.; Manning, J.J.

    1981-05-01

    This report describes the integral flux, energy spectra, and dose rate measurements made for the Exit Shield Experiment at the Oak Ridge National Laboratory Tower Shielding Facility as part of the Gas Cooled Fast Breeder Reactor program. The source was the same mockup of fuel pins used in the previous Grid Plate Shield Experiment. Two mockups of the upper axial shield were studied: one with seven subassemblies prototypic of that portion of the Exit Shield without a control rod, and another that was representative of the shield region with a control rod. The experiment was performed to provide verification of: the shield design methods, the shield effectiveness of a prototypic mockup, the analytical ability to calculate streaming effects in the presence of a control rod, and the source term bias factors for the upper plenum.

  4. Protein-induced changes in DNA structure and dynamics observed with noncovalent site-directed spin labeling and PELDOR

    PubMed Central

    Reginsson, Gunnar W.; Shelke, Sandip A.; Rouillon, Christophe; White, Malcolm F.; Sigurdsson, Snorri Th.; Schiemann, Olav

    2013-01-01

    Site-directed spin labeling and pulsed electron–electron double resonance (PELDOR or DEER) have previously been applied successfully to study the structure and dynamics of nucleic acids. Spin labeling nucleic acids at specific sites requires the covalent attachment of spin labels, which involves rather complicated and laborious chemical synthesis. Here, we use a noncovalent label strategy that bypasses the covalent labeling chemistry and show that the binding specificity and efficiency are large enough to enable PELDOR or DEER measurements in DNA duplexes and a DNA duplex bound to the Lac repressor protein. In addition, the rigidity of the label not only allows resolution of the structure and dynamics of oligonucleotides but also the determination of label orientation and protein-induced conformational changes. The results prove that this labeling strategy in combination with PELDOR has a great potential for studying both structure and dynamics of oligonucleotides and their complexes with various ligands. PMID:22941643

  5. Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field.

    PubMed

    Carmelo, J M P; Sacramento, P D; Machado, J D P; Campbell, D K

    2015-10-14

    We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the 'pseudofermion dynamical theory' (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents ζ(τ)(k) controlling the singularities for both the longitudinal (τ = l) and transverse (τ = t) dynamical structure factors for the whole momentum range k ∈ ]0,π[, in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions. PMID:26403307

  6. Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field

    NASA Astrophysics Data System (ADS)

    Carmelo, J. M. P.; Sacramento, P. D.; Machado, J. D. P.; Campbell, D. K.

    2015-10-01

    We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the ‘pseudofermion dynamical theory’ (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents {{\\zeta}τ}(k) controlling the singularities for both the longitudinal ≤ft(τ =l\\right) and transverse ≤ft(τ =t\\right) dynamical structure factors for the whole momentum range k\\in ]0,π[ , in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions.

  7. Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field.

    PubMed

    Carmelo, J M P; Sacramento, P D; Machado, J D P; Campbell, D K

    2015-10-14

    We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the 'pseudofermion dynamical theory' (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents ζ(τ)(k) controlling the singularities for both the longitudinal (τ = l) and transverse (τ = t) dynamical structure factors for the whole momentum range k ∈ ]0,π[, in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions.

  8. Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7

    NASA Astrophysics Data System (ADS)

    Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.

    2012-09-01

    Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.

  9. Decoupling a spin qubit from high-frequency Larmor dynamics of a GaAs nuclear spin bath

    NASA Astrophysics Data System (ADS)

    Malinowski, Filip K.; Martins, Frederico; Nissen, Peter D.; Rudner, Mark S.; Marcus, Charles M.; Kuemmeth, Ferdinand; Barnes, Edwin; Fallahi, Saeed; Gardner, Geoffrey C.; Manfra, Michael J.

    We present a technique of decoupling a spin qubit in a GaAs/AlGaAs heterostructure from low- and high-frequency noise arising from hyperfine interaction of electrons with nuclear spins. We use Carr-Purcell-Meiboom-Gill sequences in which we synchronize the repetition rate of π pulses to difference Larmor frequencies of 69Ga, 71Ga and 75As nuclei. This decouples the qubit both from low-frequency noise due to diffusion of nuclear spins and from noise at selected high frequencies, allowing us to apply more than a thousand π pulses in a sequence. We demonstrate a coherence time of a singlet-triplet qubit of 0.87 ms, i.e. five orders of magnitude longer than the inhomogeneous dephasing time intrinsic to GaAs. Support through IARPA-MQCO, Army Research Office, LPS-MPO-CMTC, the Villum Foundation and the Danish National Research Foundation is acknowledged.

  10. A simulation study of magnetic vortex structures and spin dynamic modes in permalloy materials

    NASA Astrophysics Data System (ADS)

    Wang, Hao

    Transverse spin wave modes of a long thin-film permalloy stripe have been studied using micromagnetic simulations and a semi-analytical theory. Lower frequency modes were found localized near the edge of the stripe and higher frequency modes exhibited a crossover property. These features result from the inhomogeneous distribution of the equilibrium magnetization and internal field across the stripe, which is adjusted by an applied field across the width of the stripe. Mode frequencies and wave profiles show distinct characteristics under different applied fields. Mode softening happens at two critical fields corresponding to a symmetry transition of the magnetic system. Spin dynamic modes of a magnetic antivortex in asteroid-shaped permalloy samples were systematically explored using micromagnetic simulations. A gyrotropic mode was found due to the shift of the antivortex from its equilibrium position. Azimuthal and radial spin wave modes have been excited by a pulsed magnetic field in different directions. Coupling between gyrotropic and azimuthal modes splits the degeneracy of paired azimuthal modes. Frequencies of the spin wave modes decrease with asteroid size and thickness while the frequency of the gyrotropic mode increases with asteroid thickness but decreases with asteroid size. The vortex dynamics of a magnetic vortex-antivortex-vortex structure in elliptical permalloy samples was studied using a theoretical model and micromagnetic simulations. Three gyrotropic modes were found to exist and each of them can be excited by a special initial configuration of core displacements. The polarizations of three cores play an important role on the mode frequencies and relative core movements in each mode. The annihilation process of a magnetic vortex pair confined in stadium-shaped permalloy samples was investigated using micromagnetic simulations. With the strength of an applied magnetic field across the width of stadia increasing, the equilibrium magnetization of

  11. Soft mode characteristics of up-up-down-down spin chains: The role of exchange interactions on lattice dynamics

    SciTech Connect

    Guo, Y. J.; Gao, Y. J.; Ge, C. N; Guo, Y. Y.; Yan, Z. B.; Liu, J.-M.

    2015-05-07

    In this work, the dynamics of a diatomic chain is investigated with ↑↑↓↓ spin order in which the dispersion relation characterizes the effect of magnetic interactions on the lattice dynamics. The optical or acoustic mode softening in the center or boundary of the Brillouin zone can be observed, indicating the transitions of ferroelectric state, antiferromagnetic state, or ferroelastic state. The coexistence of the multiferroic orders related to the ↑↑↓↓ spin order represents a type of intrinsic multiferroic with strong ferroelectric order and different microscopic mechanisms.

  12. Elasto-dynamic analysis of spinning nanodisks via a surface energy-based model

    NASA Astrophysics Data System (ADS)

    Kiani, Keivan

    2016-07-01

    Using the surface elasticity theory of Gurtin and Murdoch, in-plane vibrations of annular nanodisks due to their rotary motion are explored. By the imposition of non-classical boundary conditions on the innermost and outermost surfaces and employing Hamilton’s principle, the unknown elasto-dynamic fields of the bulk zone are determined via the finite element method. The roles of both nanodisk geometry and surface effect on the natural frequencies are addressed. Subsequently, forced vibrations of spinning nanodisks with fixed-free and free-free boundary conditions are comprehensively examined. The obtained results show that the maximum dynamic elastic fields grow in a parabolic manner as the steady angular velocity increases. By increasing the outermost radius, the maximum dynamic elastic field is magnified and the influence of the surface effect on the results reduced. This work can be considered as a pivotal step towards optimal design and dynamic analysis of nanorotors with disk-like parts, which are one of the basic building blocks of the upcoming advanced nanotechnologies.

  13. Elasto-dynamic analysis of spinning nanodisks via a surface energy-based model

    NASA Astrophysics Data System (ADS)

    Kiani, Keivan

    2016-07-01

    Using the surface elasticity theory of Gurtin and Murdoch, in-plane vibrations of annular nanodisks due to their rotary motion are explored. By the imposition of non-classical boundary conditions on the innermost and outermost surfaces and employing Hamilton’s principle, the unknown elasto-dynamic fields of the bulk zone are determined via the finite element method. The roles of both nanodisk geometry and surface effect on the natural frequencies are addressed. Subsequently, forced vibrations of spinning nanodisks with fixed–free and free–free boundary conditions are comprehensively examined. The obtained results show that the maximum dynamic elastic fields grow in a parabolic manner as the steady angular velocity increases. By increasing the outermost radius, the maximum dynamic elastic field is magnified and the influence of the surface effect on the results reduced. This work can be considered as a pivotal step towards optimal design and dynamic analysis of nanorotors with disk-like parts, which are one of the basic building blocks of the upcoming advanced nanotechnologies.

  14. Recent NASA Research on Aerodynamic Modeling of Post-Stall and Spin Dynamics of Large Transport Airplanes

    NASA Technical Reports Server (NTRS)

    Murch, Austin M.; Foster, John V.

    2007-01-01

    A simulation study was conducted to investigate aerodynamic modeling methods for prediction of post-stall flight dynamics of large transport airplanes. The research approach involved integrating dynamic wind tunnel data from rotary balance and forced oscillation testing with static wind tunnel data to predict aerodynamic forces and moments during highly dynamic departure and spin motions. Several state-of-the-art aerodynamic modeling methods were evaluated and predicted flight dynamics using these various approaches were compared. Results showed the different modeling methods had varying effects on the predicted flight dynamics and the differences were most significant during uncoordinated maneuvers. Preliminary wind tunnel validation data indicated the potential of the various methods for predicting steady spin motions.

  15. Theoretical model of dynamic spin polarization of nuclei coupled to paramagnetic point defects in diamond and silicon carbide

    NASA Astrophysics Data System (ADS)

    Ivády, Viktor; Szász, Krisztián; Falk, Abram L.; Klimov, Paul V.; Christle, David J.; Janzén, Erik; Abrikosov, Igor A.; Awschalom, David D.; Gali, Adam

    2015-09-01

    Dynamic nuclear spin polarization (DNP) mediated by paramagnetic point defects in semiconductors is a key resource for both initializing nuclear quantum memories and producing nuclear hyperpolarization. DNP is therefore an important process in the field of quantum-information processing, sensitivity-enhanced nuclear magnetic resonance, and nuclear-spin-based spintronics. DNP based on optical pumping of point defects has been demonstrated by using the electron spin of nitrogen-vacancy (NV) center in diamond, and more recently, by using divacancy and related defect spins in hexagonal silicon carbide (SiC). Here, we describe a general model for these optical DNP processes that allows the effects of many microscopic processes to be integrated. Applying this theory, we gain a deeper insight into dynamic nuclear spin polarization and the physics of diamond and SiC defects. Our results are in good agreement with experimental observations and provide a detailed and unified understanding. In particular, our findings show that the defect electron spin coherence times and excited state lifetimes are crucial factors in the entire DNP process.

  16. Magnetic shielding

    DOEpatents

    Kerns, J.A.; Stone, R.R.; Fabyan, J.

    1987-10-06

    A magnetically-conductive filler material bridges the gap between a multi-part magnetic shield structure which substantially encloses a predetermined volume so as to minimize the ingress or egress of magnetic fields with respect to that volume. The filler material includes a heavy concentration of single-magnetic-domain-sized particles of a magnetically conductive material (e.g. soft iron, carbon steel or the like) dispersed throughout a carrier material which is generally a non-magnetic material that is at least sometimes in a plastic or liquid state. The maximum cross-sectional particle dimension is substantially less than the nominal dimension of the gap to be filled. An epoxy base material (i.e. without any hardening additive) low volatility vacuum greases or the like may be used for the carrier material. The structure is preferably exposed to the expected ambient magnetic field while the carrier is in a plastic or liquid state so as to facilitate alignment of the single-magnetic-domain-sized particles with the expected magnetic field lines. 3 figs.

  17. Magnetic shielding

    DOEpatents

    Kerns, J.A.; Stone, R.R.; Fabyan, J.

    1985-02-12

    A magnetically-conductive filler material bridges the gap between a multi-part magnetic shield structure which substantially encloses a predetermined volume so as to minimize the ingress or egress of magnetic fields with respect to that volume. The filler material includes a heavy concentration of single-magnetic-domain-sized particles of a magnetically conductive material (e.g. soft iron, carbon steel or the like) dispersed throughout a carrier material which is generally a non-magnetic material that is at least sometimes in a plastic or liquid state. The maximum cross-sectional particle dimension is substantially less than the nominal dimension of the gap to be filled. An epoxy base material (i.e. without any hardening additive) low volatility vacuum greases or the like may be used for the carrier material. The structure is preferably exposed to the expected ambient field while the carrier is in a plastic or liquid state so as to facilitate alignment of the single-magnetic-domain-sized particles with the expected magnetic field lines.

  18. Magnetic shielding

    DOEpatents

    Kerns, John A.; Stone, Roger R.; Fabyan, Joseph

    1987-01-01

    A magnetically-conductive filler material bridges the gap between a multi-part magnetic shield structure which substantially encloses a predetermined volume so as to minimize the ingress or egress of magnetic fields with respect to that volume. The filler material includes a heavy concentration of single-magnetic-domain-sized particles of a magnetically conductive material (e.g. soft iron, carbon steel or the like) dispersed throughout a carrier material which is generally a non-magnetic material that is at least sometimes in a plastic or liquid state. The maximum cross-sectional particle dimension is substantially less than the nominal dimension of the gap to be filled. An epoxy base material (i.e. without any hardening additive) low volatility vacuum greases or the like may be used for the carrier material. The structure is preferably exposed to the expected ambient magnetic field while the carrier is in a plastic or liquid state so as to facilitate alignment of the single-magnetic-domain-sized particles with the expected magnetic field lines.

  19. Tuning the presence of dynamical phase transitions in a generalized X Y spin chain

    NASA Astrophysics Data System (ADS)

    Divakaran, Uma; Sharma, Shraddha; Dutta, Amit

    2016-05-01

    We study an integrable spin chain with three spin interactions and the staggered field (λ ) while the latter is quenched either slowly [in a linear fashion in time (t ) as t /τ , where t goes from a large negative value to a large positive value and τ is the inverse rate of quenching] or suddenly. In the process, the system crosses quantum critical points and gapless phases. We address the question whether there exist nonanalyticities [known as dynamical phase transitions (DPTs)] in the subsequent real-time evolution of the state (reached following the quench) governed by the final time-independent Hamiltonian. In the case of sufficiently slow quenching (when τ exceeds a critical value τ1), we show that DPTs, of the form similar to those occurring for quenching across an isolated critical point, can occur even when the system is slowly driven across more than one critical point and gapless phases. More interestingly, in the anisotropic situation we show that DPTs can completely disappear for some values of the anisotropy term (γ ) and τ , thereby establishing the existence of boundaries in the (γ -τ ) plane between the DPT and no-DPT regions in both isotropic and anisotropic cases. Our study therefore leads to a unique situation when DPTs may not occur even when an integrable model is slowly ramped across a QCP. On the other hand, considering sudden quenches from an initial value λi to a final value λf, we show that the condition for the presence of DPTs is governed by relations involving λi,λf, and γ , and the spin chain must be swept across λ =0 for DPTs to occur.

  20. Planetary dynamics from laser altimetry: Spin and tidal deformation of the Moon and Mercury

    NASA Astrophysics Data System (ADS)

    Barker, M. K.; Mazarico, E.; Smith, D. E.; Zuber, M. T.

    2015-12-01

    The dynamics of planetary bodies can provide valuable, and often unique, information on their interior structure. For instance, surface tidal deformation indicates how a body responds to the gravitational tidal forcing, and can thus give an indication of how the internal structure and temperature varies with depth. In addition, the orientation and spin rate of a planetary body are affected by its interior mass distribution and thermal evolution. In this contribution, we describe recent work to constrain the tidal deformation of the Moon and spin state and orientation of Mercury using altimetric crossovers measured by the Lunar Orbiter Laser Altimeter (LOLA) and MESSENGER Laser Altimeter (MLA). Altimetric crossovers are ideal for detecting the desired small surface changes, as they avoid the problem of aliasing topographic changes due to small-scale, unpredictable and uncorrelated, geologic relief. On the Moon, the tidal surface deformation is small (amplitude ~10 cm), but, using the highest quality LOLA crossovers, Mazarico et al. (2014) made the first measurement of the radial Love number h2 from an orbiting spacecraft. In a follow-up to that work, we are incorporating more crossovers to improve the temporal sampling of the tidal signal, thus enabling analysis of the spatial variation of the tidal amplitude, as might be expected given the thicker and cooler far side crust and the potential presence of a partial melt region below the PKT. Due to tidal torques from the Sun, Mercury experiences longitudinal librations about its 3:2 spin-orbit resonance with an amplitude of ~450 m at the equator. This amplitude is significantly larger than the geolocation uncertainty of the MLA altimetry (~10/100 m in radial/horizontal), and could, thus, be detectable from crossovers alone. However, given the sparse coverage near the equator, where the libration amplitude is largest, it may be necessary to incorporate into the analysis stereo-derived DEMs from the Mercury Dual Imaging

  1. Use of spin-labelling techniques to probe the dynamics of He(2 3S) deexcitation at solid surfaces

    NASA Astrophysics Data System (ADS)

    Dunning, F. B.; Oró, D. M.; Soletsky, P. A.; Zhang, X.; Nordlander, P.; Walters, G. K.

    1994-06-01

    Spin labelling techniques, specifically the use of electron-spin-polarized He(23 S) metastable atoms coupled with energy-resolved spin analysis of the ejected electrons, are used to investigate the dynamics of He(23 S) deexcitation at solid surfaces. Data for a clean Au(100) surface are presented that show that deexcitation occurs exclusively through resonance ionization followed by Auger neutralization. The electrons involved in Auger neutralization are observed to be correlated in spin and possible reasons for this are discussed. Results obtained at Xe and NO films adsorbed on cooled Au(100) and Cu(100) substrates, respectively, show that He(23 S) metastable atom deexcitation is analogous to gas-phase Penning ionization. Detailed differences are apparent that can be attributed to effects associated with the underlying substrate and interactions involving neighboring atoms in the film.

  2. Spin-vibronic quantum dynamics for ultrafast excited-state processes.

    PubMed

    Eng, Julien; Gourlaouen, Christophe; Gindensperger, Etienne; Daniel, Chantal

    2015-03-17

    Ultrafast intersystem crossing (ISC) processes coupled to nuclear relaxation and solvation dynamics play a central role in the photophysics and photochemistry of a wide range of transition metal complexes. These phenomena occurring within a few hundred femtoseconds are investigated experimentally by ultrafast picosecond and femtosecond transient absorption or luminescence spectroscopies, and optical laser pump-X-ray probe techniques using picosecond and femtosecond X-ray pulses. The interpretation of ultrafast structural changes, time-resolved spectra, quantum yields, and time scales of elementary processes or transient lifetimes needs robust theoretical tools combining state-of-the-art quantum chemistry and developments in quantum dynamics for solving the electronic and nuclear problems. Multimode molecular dynamics beyond the Born-Oppenheimer approximation has been successfully applied to many small polyatomic systems. Its application to large molecules containing a transition metal atom is still a challenge because of the nuclear dimensionality of the problem, the high density of electronic excited states, and the spin-orbit coupling effects. Rhenium(I) α-diimine carbonyl complexes, [Re(L)(CO)3(N,N)](n+) are thermally and photochemically robust and highly flexible synthetically. Structural variations of the N,N and L ligands affect the spectroscopy, the photophysics, and the photochemistry of these chromophores easily incorporated into a complex environment. Visible light absorption opens the route to a wide range of applications such as sensors, probes, or emissive labels for imaging biomolecules. Halide complexes [Re(X)(CO)3(bpy)] (X = Cl, Br, or I; bpy = 2,2'-bipyridine) exhibit complex electronic structure and large spin-orbit effects that do not correlate with the heavy atom effects. Indeed, the (1)MLCT → (3)MLCT intersystem crossing (ISC) kinetics is slower than in [Ru(bpy)3](2+) or [Fe(bpy)3](2+) despite the presence of a third-row transition metal

  3. Spin dynamics in the presence of competing ferromagnetic and antiferromagnetic correlations in Yb2Ti2O7

    NASA Astrophysics Data System (ADS)

    Robert, J.; Lhotel, E.; Remenyi, G.; Sahling, S.; Mirebeau, I.; Decorse, C.; Canals, B.; Petit, S.

    2015-08-01

    In this work, we show that the zero-field excitation spectra in the quantum spin ice candidate pyrochlore compound Yb2Ti2O7 is a continuum characterized by a very broad and almost flat dynamical response, which extends up to 1 -1.5 meV, coexisting or not with a quasielastic response depending on the wave vector. The spectra do not evolve between 50 mK and 2 K, indicating that the spin dynamics is only little affected by the temperature in both the short-range correlated and ordered regimes. Although classical spin dynamics simulations qualitatively capture some of the experimental observations, we show that they fail to reproduce this broad continuum. In particular, the simulations predict an energy scale twice smaller than the experimental observations. This analysis is based on a careful determination of the exchange couplings, able to reproduce both the zero-field diffuse scattering and the spin wave spectrum rising in the field polarized state. According to this analysis, Yb2Ti2O7 lies at the border between a ferro- and an antiferromagnetic phase. These results suggest that the unconventional ground state of Yb2Ti2O7 is governed by strong quantum fluctuations arising from the competition between those phases. The observed spectra may correspond to a continuum of deconfined spinons as expected in quantum spin liquids.

  4. Static and dynamic spin fluctuations in the spin glass doping regime in La sub 2-x Sr sub x CuO sub 4+y

    SciTech Connect

    Birgeneau, R.J.; Belk, N.; Kastner, M.A.; Keimer, B. . Dept. of Physics); Endoh, Y. . Dept. of Physics); Erwin, R.W. ); Shirane, G. )

    1991-01-01

    We review the results of neutron scattering studies of the static and dynamic spin fluctuations crystals of La{sub 2-x}Sr{sub x}CuO{sub 4+{delta}} in the doping regime intermediate between the Neel and superconducting regions. In this regime the in-plane resistance is linear in temperature down to {approximately}80 K with a crossover due to logarithmic conductance effects at lower temperatures. The static spin correlations are well-described by a simple model in which the inverse correlation length {kappa}(x,T) ={kappa}(x,0) + {kappa}(0,T). The most dramatic new result is the discovery by Keimer et al. that the dynamic spin fluctuations exhibit a temperature dependence which is a simple function of {omega}/T for temperatures 10 K{le}T{le}500 K for a wide range of energies. This scaling leads to a natural explanation of a variety of normal state properties of the copper oxides. 21 refs., 4 figs.

  5. Micromagnetic simulations of spin-wave normal modes and the spin-transfer-torque driven magnetization dynamics of a ferromagnetic cross

    NASA Astrophysics Data System (ADS)

    Pramanik, Tanmoy; Roy, Urmimala; Tsoi, Maxim; Register, Leonard F.; Banerjee, Sanjay K.

    2014-05-01

    We studied spin-transfer-torque (STT) switching of a cross-shaped magnetic tunnel junction in a recent report [Roy et al., J. Appl. Phys. 113, 223904 (2013)]. In that structure, the free layer is designed to have four stable energy states using the shape anisotropy of a cross. STT switching showed different regions with increasing current density. Here, we employ the micromagnetic spectral mapping technique in an attempt to understand how the asymmetry of cross dimensions and spin polarization direction of the injected current affect the magnetization dynamics. We compute spatially averaged frequency-domain spectrum of the time-domain magnetization dynamics in the presence of the current-induced STT term. At low currents, the asymmetry of polarization direction and that of the arms are observed to cause a splitting of the excited frequency modes. Higher harmonics are also observed, presumably due to spin-wave wells caused by the regions of spatially non-uniform effective magnetic field. The results could be used towards designing a multi-bit-per-cell STT-based random access memory with an improved storage density.

  6. Micromagnetic simulations of spin-wave normal modes and the spin-transfer-torque driven magnetization dynamics of a ferromagnetic cross

    SciTech Connect

    Pramanik, Tanmoy Roy, Urmimala; Register, Leonard F.; Banerjee, Sanjay K.; Tsoi, Maxim

    2014-05-07

    We studied spin-transfer-torque (STT) switching of a cross-shaped magnetic tunnel junction in a recent report [Roy et al., J. Appl. Phys. 113, 223904 (2013)]. In that structure, the free layer is designed to have four stable energy states using the shape anisotropy of a cross. STT switching showed different regions with increasing current density. Here, we employ the micromagnetic spectral mapping technique in an attempt to understand how the asymmetry of cross dimensions and spin polarization direction of the injected current affect the magnetization dynamics. We compute spatially averaged frequency-domain spectrum of the time-domain magnetization dynamics in the presence of the current-induced STT term. At low currents, the asymmetry of polarization direction and that of the arms are observed to cause a splitting of the excited frequency modes. Higher harmonics are also observed, presumably due to spin-wave wells caused by the regions of spatially non-uniform effective magnetic field. The results could be used towards designing a multi-bit-per-cell STT-based random access memory with an improved storage density.

  7. GMI in the reentrant spin-glass Fe90Zr10 alloy: Investigation of the spin dynamics in the MHz frequency regime

    NASA Astrophysics Data System (ADS)

    Ribeiro, P. R. T.; Ramírez, J. M. M.; Vidyasagar, R.; Machado, F. L. A.; Rezende, S. M.; Dahlberg, E. Dan

    2016-09-01

    Giant magnetoimpedance (GMI) in the reentrant spin-glass (SG) phase of ferromagnetic Fe90Zr10 is reported. The temperature (T) dependence of the GMI allows the investigation of the spin dynamics in the SG phase in the MHz frequency regime and thus very short relaxation times τ (˜10-8 s). The GMI shows a broad maximum around 150 K and diminishes with decreasing T below the glass temperature Tg of 15 K. The magnetic permeability data obtained from the GMI data show the general features observed in the ac magnetic susceptibility measured at lower frequencies (10 ≤ f ≤ 104 Hz), yielding values of Tf (=Tg(f)) that allow testing the validity of the power-law scaling used for describing the dynamics of SG-phases up to 15 MHz. A log-log plot of τ (=1/f) versus the reduced critical temperature shows two distinct regimes in the time-domain: (1) a critical slowing-down is observed for values τ > 3 × 10-3 s; and (2) for 7 × 10-8 ≤ τ ≤ 3 × 10-3 s. In the latter case a fitting to the power-law yields the value 7.4 for the product of the critical exponents zν, and 1.6 × 10-7 s for the microscopic relaxation time τ0. The product of the exponents is appropriate for an Ising spin glass.

  8. Electron-spin-polarized He^+ ion source for studying ion-surface interaction dynamics

    NASA Astrophysics Data System (ADS)

    Bixler, D. L.; Lancaster, J. C.; Popple, R. A.; Dunning, F. B.; Walters, G. K.

    1997-03-01

    An electron-spin-polarized He^+ ion source has been developed to study the dynamics of ion-surface interactions. The He^+ ions are produced by Penning ionization in collisions between helium metastable atoms contained in a weak rf-excited discharge. The 2^3S metastable atoms in the discharge are polarized by optical pumping using a 300 mW Ti:sapphire laser tuned to the 2^3S_1-2^3P1 (D_1) transition at 1.083μm. Spin conservation during Penning ionization results in the production of polarized He^+ ions which are extracted from the discharge through a small canal and focused on the target surface using a series of electrostatic lenses, which reduce the energy spread in the beam to ~ 3 eV through chromatic abberation. Currents of ~ 10-9 A are achieved at ion energies of >= 10 eV. The ion beam polarization is determined by allowing the beam to strike a clean Au(100) surface and observing the polarization of the ejected secondary electrons. He^+ ion polarizations of ~ 10 % are routinely obtained, and work is underway to further improve this polarization. ^*Research supported by the U.S. Department of Energy and the Robert A. Welch Foundation. DLB is the recipient of a Texaco Fellowship.

  9. Electron-spin-polarized He^+ ion source for studying ion-surface interaction dynamics

    NASA Astrophysics Data System (ADS)

    Bixler, D. L.; Lancaster, J. C.; Popple, R. A.; Dunning, F. B.; Walters, G. K.

    1997-04-01

    An electron-spin-polarized He^+ ion source has been developed to study the dynamics of ion-surface interactions. The He^+ ions are produced by Penning ionization in collisions between helium metastable atoms contained in a weak rf-excited discharge. The 2^3S metastable atoms in the discharge are polarized by optical pumping using a 300 mW Ti:sapphire laser tuned to the 2^3S_1-2^3P1 (D_1) transition at 1.083μm. Spin conservation during Penning ionization results in the production of polarized He^+ ions which are extracted from the discharge through a small canal and focused on the target surface using a series of electrostatic lenses, which reduce the energy spread in the beam to ~ 3 eV through chromatic abberation. Currents of ~ 10-9 A are achieved at ion energies of >= 10 eV. The ion beam polarization is determined by allowing the beam to strike a clean Au(100) surface and observing the polarization of the ejected secondary electrons. He^+ ion polarizations of ~ 10 % are routinely obtained, and work is underway to further improve this polarization. ^*Research supported by the U.S. Department of Energy and the Robert A. Welch Foundation.

  10. Low-energy spin dynamics of the s = 1/2 kagome system herbertsmithite.

    PubMed

    Nilsen, G J; de Vries, M A; Stewart, J R; Harrison, A; Rønnow, H M

    2013-03-13

    The low-energy (ε = ħω < 1 meV), low-temperature (T = 0.05 K) spin dynamics of the s = 1/2 kagome candidate herbertsmithite are probed in the presence of magnetic fields up to 2.5 T. The zero-field spectra reveal a very weak continuum of scattering at T = 10 K and a broad inelastic peak centred at ε(max) = 0.2 meV at lower temperatures, T < 1 K. The broad peak is found to be strongly damped, with a liquid-like structure factor implying correlations at length scales up to r = 6 Å. The field dependence of the peak appears to follow the Zeeman splitting of s = 1/2 excitations, consistent with the weakly split 'doublets' observed in low-temperature specific heat. A possible explanation of these observations is a short-range correlated state involving defect spins between the kagome planes and moments in the kagome layers.

  11. Trion fine structure and coupled spin-valley dynamics in monolayer tungsten disulfide

    NASA Astrophysics Data System (ADS)

    Plechinger, Gerd; Nagler, Philipp; Arora, Ashish; Schmidt, Robert; Chernikov, Alexey; Del Águila, Andrés Granados; Christianen, Peter C. M.; Bratschitsch, Rudolf; Schüller, Christian; Korn, Tobias

    2016-09-01

    Monolayer transition-metal dichalcogenides have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. The optical properties of these two-dimensional crystals are dominated by tightly bound electron-hole pairs (excitons) and more complex quasiparticles such as charged excitons (trions). Here we investigate monolayer WS2 samples via photoluminescence and time-resolved Kerr rotation. In photoluminescence and in energy-dependent Kerr rotation measurements, we are able to resolve two different trion states, which we interpret as intravalley and intervalley trions. Using time-resolved Kerr rotation, we observe a rapid initial valley polarization decay for the A exciton and the trion states. Subsequently, we observe a crossover towards exciton-exciton interaction-related dynamics, consistent with the formation and decay of optically dark A excitons. By contrast, resonant excitation of the B exciton transition leads to a very slow decay of the Kerr signal.

  12. Trion fine structure and coupled spin-valley dynamics in monolayer tungsten disulfide.

    PubMed

    Plechinger, Gerd; Nagler, Philipp; Arora, Ashish; Schmidt, Robert; Chernikov, Alexey; Del Águila, Andrés Granados; Christianen, Peter C M; Bratschitsch, Rudolf; Schüller, Christian; Korn, Tobias

    2016-01-01

    Monolayer transition-metal dichalcogenides have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. The optical properties of these two-dimensional crystals are dominated by tightly bound electron-hole pairs (excitons) and more complex quasiparticles such as charged excitons (trions). Here we investigate monolayer WS2 samples via photoluminescence and time-resolved Kerr rotation. In photoluminescence and in energy-dependent Kerr rotation measurements, we are able to resolve two different trion states, which we interpret as intravalley and intervalley trions. Using time-resolved Kerr rotation, we observe a rapid initial valley polarization decay for the A exciton and the trion states. Subsequently, we observe a crossover towards exciton-exciton interaction-related dynamics, consistent with the formation and decay of optically dark A excitons. By contrast, resonant excitation of the B exciton transition leads to a very slow decay of the Kerr signal. PMID:27586517

  13. Control Study for Five-axis Dynamic Spin Rig Using Magnetic Bearings

    NASA Technical Reports Server (NTRS)

    Choi, Benjamin; Johnson, Dexter; Provenza, Andrew; Morrison, Carlos; Montague, Gerald

    2003-01-01

    The NASA Glenn Research Center (GRC) has developed a magnetic bearing system for the Dynamic Spin Rig (DSR) with a fully suspended shaft that is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust magnetic bearing and the associated control system were integrated into the DSR to provide magnetic excitation as well as non-contact mag- netic suspension of a 15.88 kg (35 lb) vertical rotor with blades to induce turbomachinery blade vibration. For rotor levitation, a proportional-integral-derivative (PID) controller with a special feature for multidirectional radial excitation worked well to both support and shake the shaft with blades. However, more advanced controllers were developed and successfully tested to determine the optimal controller in terms of sensor and processing noise reduction, smaller rotor orbits, more blade vibration amplitude, and energy savings for the system. The test results of a variety of controllers that were demonstrated up to 10.000 rpm are shown. Furthermore, rotor excitation operation and conceptual study of active blade vibration control are addressed.

  14. Entanglement dynamics in Heisenberg spin chains coupled to a dissipative environment at finite temperature

    NASA Astrophysics Data System (ADS)

    Sadiek, Gehad; Almalki, Samaher

    2016-07-01

    We consider a finite one-dimensional Heisenberg XYZ spin chain under the influence of a dissipative Lindblad environment obeying the Born-Markovian constraint in presence of an external magnetic field with closed and open boundary conditions. We present an exact numerical solution for the Lindblad master equation of the system in the Liouville space. The dynamics and asymptotic behavior of the nearest-neighbor and beyond-nearest-neighbor pairwise entanglements in the system are investigated under the effect of spatial anisotropy, temperature, system size, and different initial states. The entanglements in the free spin system exhibit nonuniform oscillatory behavior that varies significantly depending on the system size, anisotropy, and initial state. The x y spatial anisotropy dictates the asymptotic behavior of the different entanglements in the system under the influence of the environment regardless of the initial state. Higher anisotropy yields higher steady-state value of the nearest-neighbor entanglement whereas a complete isotropy wipes it out. The longer range entanglements respond differently to the anisotropy variation. The anisotropy in the z direction may enhance the entanglements depending on the interplay with the magnetic field applied in the same direction. As the temperature is raised, the steady state of the short-range entanglements is found to be robust within very small nonzero temperature range that depends critically on the spatial anisotropy. Moreover, the end to end entanglement transfer time and speed through the open boundary chain vary considerably based on the degree of anisotropy and temperature of the environment.

  15. Dynamic spin-flip shot noise of mesoscopic transport through a toroidal carbon nanotube

    NASA Astrophysics Data System (ADS)

    Zhao, H. K.; Zhang, J.; Wang, J.

    2015-01-01

    The shot noise in a toroidal carbon nanotube (TCN) interferometer under the perturbation of a rotating magnetic field (RMF) has been investigated. A general shot noise formula has been derived by calculating the current correlation. It was found that photon absorption and emission induce novel features of dynamic shot noise. The oscillatory behavior of shot noise and Fano factor vary with the Aharonov-Bohm (AB) magnetic flux, and they are sensitively dependent on the Zeeman energy, frequency of RMF, and source-drain bias. By adjusting the Zeeman energy, the AB oscillation structures of shot noise and Fano factor show valley-to-peak transformation. The shot noise increases nonlinearly with increasing the Zeeman energy and photon energy. The enhancement and asymmetry of shot noise can be attributed to the spin-flip effect.

  16. Characterization of heteronuclear decoupling through proton spin dynamics in solid-state nuclear magnetic resonance spectroscopy

    NASA Astrophysics Data System (ADS)

    De Paëpe, Gaël; Eléna, Bénédicte; Emsley, Lyndon

    2004-08-01

    The work presented here aims at understanding the performance of phase modulated heteronuclear decoupling sequences such as Cosine Modulation or Two Pulse Phase Modulation. To that end we provide an analytical description of the intrinsic behavior of Cosine Modulation decoupling with respect to radio-frequency-inhomogeneity and the proton-proton dipolar coupling network. We discover through a Modulation Frame average Hamiltonian analysis that best decoupling is obtained under conditions where the heteronuclear interactions are removed but notably where homonuclear couplings are recoupled at a homonuclear Rotary Resonance (HORROR) condition in the Modulation Frame. These conclusions are supported by extensive experimental investigations, and notably through the introduction of proton nutation experiments to characterize spin dynamics in solids under decoupling conditions. The theoretical framework presented in this paper allows the prediction of the optimum parameters for a given set of experimental conditions.

  17. CP-Violation from Spin-1 Resonances in a Left-Right Dynamical Higgs Context

    NASA Astrophysics Data System (ADS)

    Ruan, Kun-Ming; Shu, Jing; Yepes, Juan

    2016-07-01

    New physics field content in the nature, more specifically, from spin-1 resonances sourced by the extension of the SM local gauge symmetry to the larger local group SU(2)L ⊗ SU(2)R ⊗ U(1)B-L, may induce CP-violation signalling NP effects from higher energy regimes. In this work we completely list and study all the CP-violating operators up to the p4-order in the Lagrangian expansion, for a non-linear left-right electroweak chiral context and coupled to a light dynamical Higgs. Heavy right handed fields can be integrated out from the physical spectrum, inducing thus a physical impact in the effective gauge couplings, fermionic electric dipole moment, and CP-violation in the decay h → ZZ* → 4l that are briefly analysed. The final relevant set of effective operators have also been identified at low energies. Supported by KITPC financial during the completion of this work

  18. Study of spin dynamics and damping on the magnetic nanowire arrays with various nanowire widths

    NASA Astrophysics Data System (ADS)

    Cho, Jaehun; Fujii, Yuya; Konioshi, Katsunori; Yoon, Jungbum; Kim, Nam-Hui; Jung, Jinyong; Miwa, Shinji; Jung, Myung-Hwa; Suzuki, Yoshishige; You, Chun-Yeol

    2016-07-01

    We investigate the spin dynamics including Gilbert damping in the ferromagnetic nanowire arrays. We have measured the ferromagnetic resonance of ferromagnetic nanowire arrays using vector-network analyzer ferromagnetic resonance (VNA-FMR) and analyzed the results with the micromagnetic simulations. We find excellent agreement between the experimental VNA-FMR spectra and micromagnetic simulations result for various applied magnetic fields. We find that the same tendency of the demagnetization factor for longitudinal and transverse conditions, Nz (Ny) increases (decreases) as increasing the nanowire width in the micromagnetic simulations while Nx is almost zero value in transverse case. We also find that the Gilbert damping constant increases from 0.018 to 0.051 as the increasing nanowire width for the transverse case, while it is almost constant as 0.021 for the longitudinal case.

  19. Vortex-induced dynamic loads on a non-spinning volleyball

    NASA Astrophysics Data System (ADS)

    Qing-ding, Wei; Rong-sheng, Lin; Zhi-jie, Liu

    1988-09-01

    An experiment on vortex-induced dynamic loads on a non-spinning Volleyball was conducted in a wind tunnel. The flow past the Volleyball was visualized, and the aerodynamic load was measured by use of a strain gauge balance. The separation on the Volleyball was measured with hot-film. The experimental results suggest that under the action of an unstable tail vortex system the separation region is changeable, and that the fluctuation of drag and lateral forces is the same order of magnitude as the mean drag, no matter whether the seam of the Volleyball is symmetric or asymmetric, with regard to the flow. Based on the experimental data a numerical simulation of Volleyball swerve motion was made.

  20. Tunable magnetization dynamics in disordered FePdPt ternary alloys: Effects of spin orbit coupling

    SciTech Connect

    Ma, L.; Fan, W. J. Chen, F. L.; Zhou, S. M.; Li, S. F.; Lai, T. S.; He, P.; Xu, X. G.; Jiang, Y.

    2014-09-21

    The magnetization dynamics of disordered Fe₀.₅(Pd{sub 1–x}Pt{sub x})₀.₅ alloy films was studied by time-resolved magneto-optical Kerr effect and ferromagnetic resonance. The intrinsic Gilbert damping parameter α₀ and the resonance linewidth change linearly with the Pt atomic concentration. In particular, the induced in-plane uniaxial anisotropy constant K{sub U} also increases for x increasing from 0 to 1. All these results can be attributed to the tuning effect of the spin orbit coupling. For the disordered ternary alloys, an approach is proposed to control the induced in-plane uniaxial anisotropy, different from conventional thermal treat methods, which is helpful to design and fabrications of spintronic devices.

  1. Magnetic Order and Spin Dynamics in a Hexagonal Rare Earth Manganite

    NASA Astrophysics Data System (ADS)

    Helton, J. S.; Singh, D. K.; Elizabeth, S.; Harikrishnan, S.; Lynn, J. W.

    2011-03-01

    Hexagonal rare earth manganites, RMn O3 R = Dy, Ho, Er, Tm, Yb, Lu, Y, or Sc), have attracted a great deal of recent attention as magnetoelectric multiferroics as most of these systems are ferroelectric at room temperature and display magnetic order below TN ~ 100 K. This magnetic order can be quite complex, as both the R and Mn ions lie on geometrically frustrated triangular lattices. DyMn O3 is typically orthorhombic, but can also be grown in the hexagonal phase; Dy 0.5 Y0.5 Mn O3 displays the hexagonal phase and is magnetically diluted at the rare earth site. We have used neutron scattering experiments to explore the magnetic structure and spin dynamics of Dy 0.5 Y0.5 Mn O3 .

  2. Dynamic selective switching in antiferromagnetically-coupled bilayers close to the spin reorientation transition

    SciTech Connect

    Fernández-Pacheco, A. Mansell, R.; Petit, D.; Lee, J. H.; Cowburn, R. P.; Ummelen, F. C.; Swagten, H. J. M.

    2014-09-01

    We have designed a bilayer synthetic antiferromagnet where the order of layer reversal can be selected by varying the sweep rate of the applied magnetic field. The system is formed by two ultra-thin ferromagnetic layers with different proximities to the spin reorientation transition, coupled antiferromagnetically using Ruderman-Kittel-Kasuya-Yosida interactions. The different dynamic magnetic reversal behavior of both layers produces a crossover in their switching fields for field rates in the kOe/s range. This effect is due to the different effective anisotropy of both layers, added to an appropriate asymmetric antiferromagnetic coupling between them. Field-rate controlled selective switching of perpendicular magnetic anisotropy layers as shown here can be exploited in sensing and memory applications.

  3. Complex ordering in spin networks: Critical role of adaptation rate for dynamically evolving interactions

    NASA Astrophysics Data System (ADS)

    Pathak, Anand; Sinha, Sitabhra

    2015-09-01

    Many complex systems can be represented as networks of dynamical elements whose states evolve in response to interactions with neighboring elements, noise and external stimuli. The collective behavior of such systems can exhibit remarkable ordering phenomena such as chimera order corresponding to coexistence of ordered and disordered regions. Often, the interactions in such systems can also evolve over time responding to changes in the dynamical states of the elements. Link adaptation inspired by Hebbian learning, the dominant paradigm for neuronal plasticity, has been earlier shown to result in structural balance by removing any initial frustration in a system that arises through conflicting interactions. Here we show that the rate of the adaptive dynamics for the interactions is crucial in deciding the emergence of different ordering behavior (including chimera) and frustration in networks of Ising spins. In particular, we observe that small changes in the link adaptation rate about a critical value result in the system exhibiting radically different energy landscapes, viz., smooth landscape corresponding to balanced systems seen for fast learning, and rugged landscapes corresponding to frustrated systems seen for slow learning.

  4. Hybrid Molecular and Spin Dynamics Simulations for Ensembles of Magnetic Nanoparticles for Magnetoresistive Systems

    PubMed Central

    Teich, Lisa; Schröder, Christian

    2015-01-01

    The development of magnetoresistive sensors based on magnetic nanoparticles which are immersed in conductive gel matrices requires detailed information about the corresponding magnetoresistive properties in order to obtain optimal sensor sensitivities. Here, crucial parameters are the particle concentration, the viscosity of the gel matrix and the particle structure. Experimentally, it is not possible to obtain detailed information about the magnetic microstructure, i.e., orientations of the magnetic moments of the particles that define the magnetoresistive properties, however, by using numerical simulations one can study the magnetic microstructure theoretically, although this requires performing classical spin dynamics and molecular dynamics simulations simultaneously. Here, we present such an approach which allows us to calculate the orientation and the trajectory of every single magnetic nanoparticle. This enables us to study not only the static magnetic microstructure, but also the dynamics of the structuring process in the gel matrix itself. With our hybrid approach, arbitrary sensor configurations can be investigated and their magnetoresistive properties can be optimized. PMID:26580623

  5. Probing the holographic principle using dynamical gauge effects from open spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    Zhao, Jianshi; Price, Craig; Liu, Qi; Gemelke, Nathan

    2016-05-01

    Dynamical gauge fields result from locally defined symmetries and an effective over-labeling of quantum states. Coupling atoms weakly to a reservoir of laser modes can create an effective dynamical gauge field purely due to the disregard of information in the optical states. Here we report measurements revealing effects of open spin-orbit coupling in a system where an effective model can be formed from a non-abelian SU(2) × U(1) field theory following the Yang-Mills construct. Forming a close analogy to dynamical gauge effects in quantum chromodynamics, we extract a measure of atomic motion which reveals the analog of a closing mass gap for the relevant gauge boson, shedding insight on long standing open problems in gauge-fixing scale anomalies. Using arguments following the holographic principle, we measure scaling relations which can be understood by quantifying information present in the local potential. New prospects using these techniques for developing fractionalization of multi-particle and macroscopic systems using dissipative and non-abelian gauge fields will also be discussed. We acknowledge support from NSF Award No. 1068570, and the Charles E. Kaufman Foundation.

  6. Overlap and activity glass transitions in plaquette spin models with hierarchical dynamics

    NASA Astrophysics Data System (ADS)

    Turner, Robert M.; Jack, Robert L.; Garrahan, Juan P.

    2015-08-01

    We consider thermodynamic and dynamic phase transitions in plaquette spin models of glasses. The thermodynamic transitions involve coupled (annealed) replicas of the model. We map these coupled-replica systems to a single replica in a magnetic field, which allows us to analyze the resulting phase transitions in detail. For the triangular plaquette model (TPM), we find for the coupled-replica system a phase transition between high- and low-overlap phases, occurring at a coupling ɛ*(T ) , which vanishes in the low-temperature limit. Using computational path sampling techniques, we show that a single TPM also displays "space-time" transitions between active and inactive dynamical phases. These first-order dynamical transitions occur at a critical counting field sc(T ) ≳0 that appears to vanish at zero temperature in a manner reminiscent of the thermodynamic overlap transition. In order to extend the ideas to three dimensions, we introduce the square pyramid model, which also displays both overlap and activity transitions. We discuss a possible common origin of these various phase transitions, based on long-lived (metastable) glassy states.

  7. Dynamic and static fluctuations in polymer gels studied by neutron spin-echo

    NASA Astrophysics Data System (ADS)

    Kanaya, T.; Takahashi, N.; Nishida, K.; Seto, H.; Nagao, M.; Takeba, Y.

    2006-11-01

    We report neutron spin-echo measurements on three types of poly(vinyl alcohol) (PVA) gels. The first is PVA gel in a mixture of dimethyl sulfoxide (DMSO) and water with volume ratio 60/40, the second is PVA gel in an aqueous borax solution and the third is chemically cross-linked PVA gel. The observed normalized intermediate scattering functions I( Q, t)/ I( Q,0) were very different among them. The I( Q, t)/ I( Q,0) of the first and third gels showed a non-decaying component in addition to a decaying component, but the second one did not have the non-decaying one. This clearly indicates that the fluctuations in the first and third PVA gels consist of static and dynamic fluctuations whereas the second PVA gel does include only the dynamic fluctuations. The dynamic and static fluctuations of the PVA gels were analyzed in terms of a restricted motion in the gel network and the Zimm motion, respectively.

  8. Probing Structure and Dynamics of Protein Assemblies by Magic Angle Spinning NMR Spectroscopy

    PubMed Central

    Yan, Si; Suiter, Christopher L.; Hou, Guangjin; Zhang, Huilan; Polenova, Tatyana

    2013-01-01

    CONSPECTUS In living organisms, biological molecules often organize into multi-component complexes. Such assemblies consist of various proteins and carry out essential functions, ranging from cell division, transport, and energy transduction to catalysis, signaling, and viral infectivity. To understand the biological functions of these assemblies, in both healthy and disease states, researchers need to study their three-dimensional architecture and molecular dynamics. To date, the large size, the lack of inherent long-range order, and insolubility have made atomic-resolution studies of many protein assemblies challenging or impractical using traditional structural biology methods such as X-ray diffraction and solution NMR spectroscopy. In the past ten years, we have focused our work on the development and application of magic angle spinning solid-state NMR (MAS NMR) methods to characterize large protein assemblies at atomic-level resolution. In this Account, we discuss the rapid progress in the field of MAS NMR spectroscopy, citing work from our laboratory and others on methodological developments that have facilitated the in-depth analysis of biologically important protein assemblies. We emphasize techniques that yield enhanced sensitivity and resolution, such as fast MAS (spinning frequencies of 40 kHz and above) and non-uniform sampling protocols for data acquisition and processing. We also discuss the experiments for gaining distance restraints and for recoupling anisotropic tensorial interactions under fast MAS conditions. We give an overview of sample preparation approaches when working with protein assemblies. Following the overview of contemporary MAS NMR methods, we present case studies into the structure and dynamics of two classes of biological systems under investigation in our laboratory. We will first turn our attention to cytoskeletal microtubule motor proteins including mammalian dynactin and dynein light chain 8. We will then discuss protein

  9. Fully Suspended, Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig With Forced Excitation

    NASA Technical Reports Server (NTRS)

    Morrison, Carlos R.; Provenza, Andrew; Kurkov, Anatole; Montague, Gerald; Duffy, Kirsten; Mehmed, Oral; Johnson, Dexter; Jansen, Ralph

    2004-01-01

    The Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig, a significant advancement in the Dynamic Spin Rig (DSR), is used to perform vibration tests of turbomachinery blades and components under rotating and nonrotating conditions in a vacuum. The rig has as its critical components three magnetic bearings: two heteropolar radial active magnetic bearings and a magnetic thrust bearing. The bearing configuration allows full vertical rotor magnetic suspension along with a feed-forward control feature, which will enable the excitation of various natural blade modes in bladed disk test articles. The theoretical, mechanical, electrical, and electronic aspects of the rig are discussed. Also presented are the forced-excitation results of a fully levitated, rotating and nonrotating, unbladed rotor and a fully levitated, rotating and nonrotating, bladed rotor in which a pair of blades was arranged 180 degrees apart from each other. These tests include the bounce mode excitation of the rotor in which the rotor was excited at the blade natural frequency of 144 Hz. The rotor natural mode frequency of 355 Hz was discerned from the plot of acceleration versus frequency. For nonrotating blades, a blade-tip excitation amplitude of approximately 100 g/A was achieved at the first-bending critical (approximately 144 Hz) and at the first-torsional and second-bending blade modes. A blade-tip displacement of 70 mils was achieved at the first-bending critical by exciting the blades at a forced-excitation phase angle of 908 relative to the vertical plane containing the blades while simultaneously rotating the shaft at 3000 rpm.

  10. Quantum-tunneling dynamics of a spin-polarized Fermi gas in a double-well potential

    SciTech Connect

    Salasnich, L.; Mazzarella, G.; Toigo, F.; Salerno, M.

    2010-02-15

    We study the exact dynamics of a one-dimensional spin-polarized gas of fermions in a double-well potential at zero and finite temperature. Despite the system being made of noninteracting fermions, its dynamics can be quite complex, showing strongly aperiodic spatio-temporal patterns during the tunneling. The extension of these results to the case of mixtures of spin-polarized fermions interacting with self-trapped Bose-Einstein condensates (BECs) at zero temperature is considered as well. In this case we show that the fermionic dynamics remains qualitatively similar to that observed in the absence of BEC but with the Rabi frequencies of fermionic excited states explicitly depending on the number of bosons and on the boson-fermion interaction strength. From this, the possibility of controlling quantum fermionic dynamics by means of Feshbach resonances is suggested.

  11. Advanced Multifunctional MMOD Shield: Radiation Shielding Assessment

    NASA Technical Reports Server (NTRS)

    Rojdev, Kristina; Christiansen, Eric

    2013-01-01

    As NASA is looking to explore further into deep space, multifunctional materials are a necessity for decreasing complexity and mass. One area where multifunctional materials could be extremely beneficial is in the micrometeoroid orbital debris (MMOD) shield. A typical MMOD shield on the International Space Station (ISS) is a stuffed whipple shield consisting of multiple layers. One of those layers is the thermal blanket, or multi-layer insulation (MLI). Increasing the MMOD effectiveness of MLI blankets, while still preserving their thermal capabilities, could allow for a less massive MMOD shield. Thus, a study was conducted to evaluate a concept MLI blanket for an MMOD shield. In conjunction, this MLI blanket and the subsequent MMOD shield was also evaluated for its radiation shielding effectiveness towards protecting crew. The overall MMOD shielding system using the concept MLI blanket proved to only have a marginal increase in the radiation mitigating properties. Therefore, subsequent analysis was performed on various conceptual MMOD shields to determine the combination of materials that may prove superior for radiation mitigating purposes. The following paper outlines the evaluations performed and discusses the results and conclusions of this evaluation for radiation shielding effectiveness.

  12. Ultrafast electronic and spin dynamics in thin iron films: electron-magnon and electron-phonon interactions

    NASA Astrophysics Data System (ADS)

    Carpene, E.; Mancini, E.; Dallera, C.; Brenna, M.; Puppin, E.; De Silvestri, S.

    The electronic and spin dynamics in thin iron films have been investigated by means of time-resolved reflectivity and magneto-optical Kerr effect. The electron-magnon and the electron-phonon coupling times are extrapolated and their influence is discussed.

  13. Mapping membrane protein backbone dynamics: a comparison of site-directed spin labeling with NMR 15N-relaxation measurements.

    PubMed

    Lo, Ryan H; Kroncke, Brett M; Solomon, Tsega L; Columbus, Linda

    2014-10-01

    The ability to detect nanosecond backbone dynamics with site-directed spin labeling (SDSL) in soluble proteins has been well established. However, for membrane proteins, the nitroxide appears to have more interactions with the protein surface, potentially hindering the sensitivity to backbone motions. To determine whether membrane protein backbone dynamics could be mapped with SDSL, a nitroxide was introduced at 55 independent sites in a model polytopic membrane protein, TM0026. Electron paramagnetic resonance spectral parameters were compared with NMR (15)N-relaxation data. Sequential scans revealed backbone dynamics with the same trends observed for the R1 relaxation rate, suggesting that nitroxide dynamics remain coupled to the backbone on membrane proteins.

  14. Spin dynamics in the modulation frame: application to homonuclear recoupling in magic angle spinning solid-state NMR.

    PubMed

    De Paëpe, Gaël; Lewandowski, Józef R; Griffin, Robert G

    2008-03-28

    We introduce a family of solid-state NMR pulse sequences that generalizes the concept of second averaging in the modulation frame and therefore provides a new approach to perform magic angle spinning dipolar recoupling experiments. Here, we focus on two particular recoupling mechanisms-cosine modulated rotary resonance (CMpRR) and cosine modulated recoupling with isotropic chemical shift reintroduction (COMICS). The first technique, CMpRR, is based on a cosine modulation of the rf phase and yields broadband double-quantum (DQ) (13)C recoupling using >70 kHz omega(1,C)/2pi rf field for the spinning frequency omega(r)/2=10-30 kHz and (1)H Larmor frequency omega(0,H)/2pi up to 900 MHz. Importantly, for p>or=5, CMpRR recouples efficiently in the absence of (1)H decoupling. Extension to lower p values (3.5spinning frequencies is possible using low power (1)H irradiation (<0.25 omega(r)/2pi). This phenomenon is explained through higher order cross terms including a homonuclear third spin assisted recoupling mechanism among protons. CMpRR mitigates the heating effects of simultaneous high power (13)C recoupling and (1)H decoupling. The second technique, COMICS, involves low power (13)C irradiation that induces simultaneous recoupling of the (13)C DQ dipolar and isotropic chemical shift terms. In contrast to CMpRR, where the DQ bandwidth (approximately 30 kHz at omega(0,H)/2pi=750 MHz) covers the entire (13)C spectral width, COMICS recoupling, through the reintroduction of the isotropic chemical shift, is selective with respect to the carrier frequency, having a typical bandwidth of approximately 100 Hz. This approach is intended as a general frequency selective method circumventing dipolar truncation (supplementary to R(2) experiments). These new gamma-encoded sequences with attenuated rf requirements extend the applicability of homonuclear recoupling techniques to new regimes--high spinning and Larmor frequencies--and therefore should be of major

  15. Exploratory Environmental Tests of Several Heat Shields

    NASA Technical Reports Server (NTRS)

    Goodman, George P.; Betts, John, Jr.

    1961-01-01

    Exploratory tests have been conducted with several conceptual radiative heat shields of composite construction. Measured transient temperature distributions were obtained for a graphite heat shield without insulation and with three types of insulating materials, and for a metal multipost heat shield, at surface temperatures of approximately 2,000 F and 1,450 F, respectively, by use of a radiant-heat facility. The graphite configurations suffered loss of surface material under repeated irradiation. Temperature distribution calculated for the metal heat shield by a numerical procedure was in good agreement with measured data. Environmental survival tests of the graphite heat shield without insulation, an insulated multipost heat shield, and a stainless-steel-tile heat shield were made at temperatures of 2,000 F and dynamic pressures of approximately 6,000 lb/sq ft, provided by an ethylene-heated jet operating at a Mach number of 2.0 and sea-level conditions. The graphite heat shield survived the simulated aerodynamic heating and pressure loading. A problem area exists in the design and materials for heat-resistant fasteners between the graphite shield and the base structure. The insulated multipost heat shield was found to be superior to the stainless-steel-tile heat shield in retarding heat flow. Over-lapped face-plate joints and surface smoothness of the insulated multi- post heat shield were not adversely affected by the test environment. The graphite heat shield without insulation survived tests made in the acoustic environment of a large air jet. This acoustic environment is random in frequency and has an overall noise level of 160 decibels.

  16. Materials optimization and ghz spin dynamics of metallic ferromagnetic thin film heterostructures

    NASA Astrophysics Data System (ADS)

    Cheng, Cheng

    Metallic ferromagnetic (FM) thin film heterostructures play an important role in emerging magnetoelectronic devices, which introduce the spin degree of freedom of electrons into conventional charge-based electronic devices. As the majority of magnetoelectronic devices operate in the GHz frequency range, it is critical to understand the high-frequency magnetization dynamics in these structures. In this thesis, we start with the static magnetic properties of FM thin films and their optimization via the field-sputtering process incorporating a specially designed in-situ electromagnet. We focus on the origins of anisotropy and hysteresis/coercivity in soft magnetic thin films, which are most relevant to magentic susceptibility and power dissipation in applications in the sub-GHz frequency regime, such as magnetic-core integrated inductors. Next we explore GHz magnetization dynamics in thin-film heterostructures, both in semi-infinite samples and confined geometries. All investigations are rooted in the Landau-Lifshitz-Gilbert (LLG) equation, the equation of motion for magnetization. The phenomenological Gilbert damping parameter in the LLG equation has been interpreted, since the 1970's, in terms of the electrical resistivity. We present the first interpretation of the size effect in Gilbert damping in single metallic FM films based on this electron theory of damping. The LLG equation is intrinsically nonlinear, which provides possibilities for rf signal processing. We analyze the frequency doubling effect at small-angle magnetization precession from the first-order expansion of the LLG equation, and demonstrate second harmonic generation from Ni81 Fe19 (Permalloy) thin film under ferromagnetic resonance (FMR), three orders of magnitude more efficient than in ferrites traditionally used in rf devices. Though the efficiency is less than in semiconductor devices, we provide field- and frequency-selectivity in the second harmonic generation. To address further the

  17. Dynamic creation of a topologically-ordered Hamiltonian using spin-pulse control in the Heisenberg model

    PubMed Central

    Tanamoto, Tetsufumi; Ono, Keiji; Liu, Yu-xi; Nori, Franco

    2015-01-01

    Hamiltonian engineering is an important approach for quantum information processing, when appropriate materials do not exist in nature or are unstable. So far there is no stable material for the Kitaev spin Hamiltonian with anisotropic interactions on a honeycomb lattice, which plays a crucial role in the realization of both Abelian and non-Abelian anyons. Here, we show two methods to dynamically realize the Kitaev spin Hamiltonian from the conventional Heisenberg spin Hamiltonian using pulse-control techniques based on the Baker-Campbell-Hausdorff (BCH) formula. In the first method, the Heisenberg interaction is changed into Ising interactions in the first process of the pulse sequence. In the next process of the first method, we transform them to a desirable anisotropic Kitaev spin Hamiltonian. In the second more efficient method, we show that if we carefully design two-dimensional pulses that vary depending on the qubit location, we can obtain the desired Hamiltonian in only one step of applying the BCH formula. As an example, we apply our methods to spin qubits based on quantum dots, in which the effects of both the spin-orbit interaction and the hyperfine interaction are estimated. PMID:26081899

  18. Spins Dynamics in a Dissipative Environment: Hierarchal Equations of Motion Approach Using a Graphics Processing Unit (GPU).

    PubMed

    Tsuchimoto, Masashi; Tanimura, Yoshitaka

    2015-08-11

    A system with many energy states coupled to a harmonic oscillator bath is considered. To study quantum non-Markovian system-bath dynamics numerically rigorously and nonperturbatively, we developed a computer code for the reduced hierarchy equations of motion (HEOM) for a graphics processor unit (GPU) that can treat the system as large as 4096 energy states. The code employs a Padé spectrum decomposition (PSD) for a construction of HEOM and the exponential integrators. Dynamics of a quantum spin glass system are studied by calculating the free induction decay signal for the cases of 3 × 2 to 3 × 4 triangular lattices with antiferromagnetic interactions. We found that spins relax faster at lower temperature due to transitions through a quantum coherent state, as represented by the off-diagonal elements of the reduced density matrix, while it has been known that the spins relax slower due to suppression of thermal activation in a classical case. The decay of the spins are qualitatively similar regardless of the lattice sizes. The pathway of spin relaxation is analyzed under a sudden temperature drop condition. The Compute Unified Device Architecture (CUDA) based source code used in the present calculations is provided as Supporting Information . PMID:26574467

  19. Dynamic nuclear polarization enhanced nuclear magnetic resonance and electron spin resonance studies of hydration and local water dynamics in micelle and vesicle assemblies.

    PubMed

    McCarney, Evan R; Armstrong, Brandon D; Kausik, Ravinath; Han, Songi

    2008-09-16

    We present a unique analysis tool for the selective detection of local water inside soft molecular assemblies (hydrophobic cores, vesicular bilayers, and micellar structures) suspended in bulk water. Through the use of dynamic nuclear polarization (DNP), the (1)H NMR signal of water is amplified, as it interacts with stable radicals that possess approximately 658 times higher spin polarization. We utilized stable nitroxide radicals covalently attached along the hydrophobic tail of stearic acid molecules that incorporate themselves into surfactant-based micelle or vesicle structures. Here, we present a study of local water content and fluid viscosity inside oleate micelles and vesicles and Triton X-100 micelles to serve as model systems for soft molecular assemblies. This approach is unique because the amplification of the NMR signal is performed in bulk solution and under ambient conditions with site-specific spin labels that only detect the water that is directly interacting with the localized spin labels. Continuous wave (cw) electron spin resonance (ESR) analysis provides rotational dynamics of the spin-labeled molecular chain segments and local polarity parameters that can be related to hydration properties, whereas we show that DNP-enhanced (1)H NMR analysis of fluid samples directly provides translational water dynamics and permeability of the local environment probed by the spin label. Our technique therefore has the potential to become a powerful analysis tool, complementary to cw ESR, to study hydration characteristics of surfactant assemblies, lipid bilayers, or protein aggregates, where water dynamics is a key parameter of their structure and function. In this study, we find that there is significant penetration of water inside the oleate micelles with a higher average local water viscosity (approximately 1.8 cP) than in bulk water, and Triton X-100 micelles and oleate vesicle bilayers mostly exclude water while allowing for considerable surfactant chain

  20. spin pumping occurred under nonlinear spin precession

    NASA Astrophysics Data System (ADS)

    Zhou, Hengan; Fan, Xiaolong; Ma, Li; Zhou, Shiming; Xue, Desheng

    Spin pumping occurs when a pure-spin current is injected into a normal metal thin layer by an adjacent ferromagnetic metal layer undergoing ferromagnetic resonance, which can be understood as the inverse effect of spin torque, and gives access to the physics of magnetization dynamics and damping. An interesting question is that whether spin pumping occurring under nonlinear spin dynamics would differ from linear case. It is known that nonlinear spin dynamics differ distinctly from linear response, a variety of amplitude dependent nonlinear effect would present. It has been found that for spin precession angle above a few degrees, nonlinear damping term would present and dominated the dynamic energy/spin-moment dissipation. Since spin pumping are closely related to the damping process, it is interesting to ask whether the nonlinear damping term could be involved in spin pumping process. We studied the spin pumping effect occurring under nonlinear spin precession. A device which is a Pt/YIG microstrip coupled with coplanar waveguide was used. High power excitation resulted in spin precession entering in a nonlinear regime. Foldover resonance lineshape and nonlinear damping have been observed. Based on those nonlinear effects, we determined the values of the precession cone angles, and the maximum cone angle can reach a values as high as 21.5 degrees. We found that even in nonlinear regime, spin pumping is still linear, which means the nonlinear damping and foldover would not affect spin pumping process.