Prebiotic chemistry in clouds

NASA Technical Reports Server (NTRS)

Oberbeck, Verne R.; Marshall, John; Shen, Thomas

1991-01-01

The chemical evolution hypothesis of Woese (1979), according to which prebiotic reactions occurred rapidly in droplets in giant atmospheric reflux columns was criticized by Scherer (1985). This paper proposes a mechanism for prebiotic chemistry in clouds that answers Scherer's concerns and supports Woese's hypothesis. According to this mechanism, rapid prebiotic chemical evolution was facilitated on the primordial earth by cycles of condensation and evaporation of cloud drops containing clay condensation nuclei and nonvolatile monomers. For example, amino acids supplied by, or synthesized during entry of meteorites, comets, and interplanetary dust, would have been scavenged by cloud drops containing clay condensation nuclei and would be polymerized within cloud systems during cycles of condensation, freezing, melting, and evaporation of cloud drops.

Nitric Acid Uptake on Subtropical Cirrus Cloud Particles

NASA Technical Reports Server (NTRS)

2004-01-01

The redistribution of HNO3 via uptake and sedimentation by cirrus cloud particles is considered an important term in the upper tropospheric budget of reactive nitrogen. Numerous cirrus cloud encounters by the NASA WB-57F high-altitude research aircraft during CRYSTAL-FACE were accompanied by the observation of condensed-phase HNO3 with the NOAA chemical ionization mass spectrometer. The instrument measures HNO3 with two independent channels of detection connected to separate forward- and downward-facing inlets that allow a determination of the amount of HNO3 condensed on ice particles. Subtropical cirrus clouds, as indicated by the presence of ice particles, were observed coincident with condensed-phase HNO3 at temperatures of 197 K - 224 K and pressures of 122 hPa - 224 hPa. Maximum levels of condensed-phase HNO3 approached the gas-phase equivalent of 0.8 ppbv. Ice particle surface coverages as high as 1.4- 10(exp 14) molecules/sq cm were observed. A dissociative Langmuir adsorption model, when using an empirically derived HNO3 adsorption enthalpy of -11.0 kcal/mol, effectively describes the observed molecular coverages to within a factor of 5. The percentage of total HNO3 in the condensed phase ranged from near zero to 100% in the observed cirrus clouds. With volume-weighted mean particle diameters up to 700 pm and particle fall velocities up to 10 m/s, some observed clouds have significant potential to redistribute HNO3 in the upper troposphere.

Parameterization of bulk condensation in numerical cloud models

NASA Technical Reports Server (NTRS)

Kogan, Yefim L.; Martin, William J.

1994-01-01

The accuracy of the moist saturation adjustment scheme has been evaluated using a three-dimensional explicit microphysical cloud model. It was found that the error in saturation adjustment depends strongly on the Cloud Condensation Nucleii (CCN) concentration in the ambient atmosphere. The scheme provides rather accurate results in the case where a sufficiently large number of CCN (on the order of several hundred per cubic centimeter) is available. However, under conditions typical of marine stratocumulus cloud layers with low CCN concentration, the error in the amounts of condensed water vapor and released latent heat may be as large as 40%-50%. A revision of the saturation adjustment scheme is devised that employs the CCN concentration, dynamical supersaturation, and cloud water content as additional variables in the calculation of the condensation rate. The revised condensation model reduced the error in maximum updraft and cloud water content in the climatically significant case of marine stratocumulus cloud layers by an order of magnitude.

Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers

PubMed Central

Rosenfeld, Daniel; Zheng, Youtong; Hashimshoni, Eyal; Pöhlker, Mira L.; Jefferson, Anne; Pöhlker, Christopher; Yu, Xing; Zhu, Yannian; Liu, Guihua; Yue, Zhiguo; Fischman, Baruch; Li, Zhanqing; Giguzin, David; Goren, Tom; Artaxo, Paulo; Pöschl, Ulrich

2016-01-01

Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities (Wb). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and Wb of boundary layer convective clouds from an operational polar orbiting weather satellite. Our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation (S) is determined by Wb and the satellite-retrieved cloud base drop concentrations (Ndb), which is the same as CCN(S). Validation against ground-based CCN instruments at Oklahoma, at Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of ±25% to ±30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semitransparent cirrus. The limitation for small solar backscattering angles of <25° restricts the satellite coverage to ∼25% of the world area in a single day. PMID:26944081

Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers.

PubMed

Rosenfeld, Daniel; Zheng, Youtong; Hashimshoni, Eyal; Pöhlker, Mira L; Jefferson, Anne; Pöhlker, Christopher; Yu, Xing; Zhu, Yannian; Liu, Guihua; Yue, Zhiguo; Fischman, Baruch; Li, Zhanqing; Giguzin, David; Goren, Tom; Artaxo, Paulo; Barbosa, Henrique M J; Pöschl, Ulrich; Andreae, Meinrat O

2016-05-24

Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities (Wb). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and Wb of boundary layer convective clouds from an operational polar orbiting weather satellite. Our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation (S) is determined by Wb and the satellite-retrieved cloud base drop concentrations (Ndb), which is the same as CCN(S). Validation against ground-based CCN instruments at Oklahoma, at Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of ±25% to ±30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semitransparent cirrus. The limitation for small solar backscattering angles of <25° restricts the satellite coverage to ∼25% of the world area in a single day.

Cloud condensation nucleus-sulfate mass relationship and cloud albedo

NASA Technical Reports Server (NTRS)

Hegg, Dean A.

1994-01-01

Analysis of previously published, simultaneous measurements of cloud condensation nucleus number concentration and sulfate mass concentration suggest a nonlinear relationship between the two variables. This nonlinearity reduces the sensitivity of cloud albedo to changes in the sulfur cycle.

Effects of Latent Heating on Atmospheres of Brown Dwarfs and Directly Imaged Planets

NASA Astrophysics Data System (ADS)

Tan, Xianyu; Showman, Adam P.

2017-02-01

The growing number of observations of brown dwarfs (BDs) has provided evidence for strong atmospheric circulation on these objects. Directly imaged planets share similar observations and can be viewed as low-gravity versions of BDs. Vigorous condensate cycles of chemical species in their atmospheres are inferred by observations and theoretical studies, and latent heating associated with condensation is expected to be important in shaping atmospheric circulation and influencing cloud patchiness. We present a qualitative description of the mechanisms by which condensational latent heating influences circulation, and then illustrate them using an idealized general circulation model that includes a condensation cycle of silicates with latent heating and molecular weight effect due to the rainout of the condensate. Simulations with conditions appropriate for typical T dwarfs exhibit the development of localized storms and east-west jets. The storms are spatially inhomogeneous, evolving on a timescale of hours to days and extending vertically from the condensation level to the tropopause. The fractional area of the BD covered by active storms is small. Based on a simple analytic model, we quantitatively explain the area fraction of moist plumes and show its dependence on the radiative timescale and convective available potential energy (CAPE). We predict that if latent heating dominates cloud formation processes, the fractional coverage area of clouds decreases as the spectral type goes through the L/T transition from high to lower effective temperature. This is a natural consequence of the variation of the radiative timescale and CAPE with the spectral type.

Nitric Acid Uptake on Subtropical Cirrus Cloud Particles

NASA Technical Reports Server (NTRS)

Popp, P. J.; Gao, R. S.; Marcy, T. P.; Fahey, D. W.; Hudson, P. K.; Thompson, T. L.; Kaercher, B.; Ridley, B. A.; Weinheimer, A. J.; Knapp, D. J.;

Josephson effects in a Bose–Einstein condensate of magnons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Troncoso, Roberto E., E-mail: r.troncoso.c@gmail.com; Departamento de Física, Facultad de Ciencias Físicas y Matemáticas, Universidad de Chile, Casilla 487-3, Santiago; Núñez, Álvaro S., E-mail: alnunez@dfi.uchile.cl

A phenomenological theory is developed, that accounts for the collective dynamics of a Bose–Einstein condensate of magnons. In terms of such description we discuss the nature of spontaneous macroscopic interference between magnon clouds, highlighting the close relation between such effects and the well known Josephson effects. Using those ideas, we present a detailed calculation of the Josephson oscillations between two magnon clouds, spatially separated in a magnonic Josephson junction. -- Highlights: •We presented a theory that accounts for the collective dynamics of a magnon-BEC. •We discuss the nature of macroscopic interference between magnon-BEC clouds. •We remarked the close relation betweenmore » the above phenomena and Josephson’s effect. •We remark the distinctive oscillations that characterize the Josephson oscillations.« less

Condensed-Phase Nitric Acid in a Tropical Subvisible Cirrus Cloud

NASA Technical Reports Server (NTRS)

Popp, P. J.; Marcy, T. P.; Watts, O. A.; Gao, R. S.; Fahey, D. W.; Weinstock, E. M.; Smith, J. B.; Herman, R. L.; Tropy, R. F.; Webster, C. r.;

Cloud condensation nuclei near marine cumulus

NASA Technical Reports Server (NTRS)

Hudson, James G.

1993-01-01

Extensive airborne measurements of cloud condensation nucleus (CCN) spectra and condensation nuclei below, in, between, and above the cumulus clouds near Hawaii point to important aerosol-cloud interactions. Consistent particle concentrations of 200/cu cm were found above the marine boundary layer and within the noncloudy marine boundary layer. Lower and more variable CCN concentrations within the cloudy boundary layer, especially very close to the clouds, appear to be a result of cloud scavenging processes. Gravitational coagulation of cloud droplets may be the principal cause of this difference in the vertical distribution of CCN. The results suggest a reservoir of CCN in the free troposphere which can act as a source for the marine boundary layer.

Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rosenfeld, Daniel; Zheng, Youtong; Hashimshoni, Eyal

Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities ( Wb). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and Wb of boundary layer convective clouds from an operational polar orbiting weather satellite. In this paper, our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation ( S) is determined by Wb and the satellite-retrieved cloud basemore » drop concentrations ( Ndb), which is the same as CCN(S). Validation against ground-based CCN instruments at Oklahoma, at Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of ±25% to ±30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semitransparent cirrus. Finally, the limitation for small solar backscattering angles of <25° restricts the satellite coverage to ~25% of the world area in a single day.« less

Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers

DOE PAGES

Rosenfeld, Daniel; Zheng, Youtong; Hashimshoni, Eyal; ...

2016-03-04

Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities ( Wb). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and Wb of boundary layer convective clouds from an operational polar orbiting weather satellite. In this paper, our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation ( S) is determined by Wb and the satellite-retrieved cloud basemore » drop concentrations ( Ndb), which is the same as CCN(S). Validation against ground-based CCN instruments at Oklahoma, at Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of ±25% to ±30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semitransparent cirrus. Finally, the limitation for small solar backscattering angles of <25° restricts the satellite coverage to ~25% of the world area in a single day.« less

Femtosecond laser filament induced condensation and precipitation in a cloud chamber

PubMed Central

Ju, Jingjing; Liu, Jiansheng; Liang, Hong; Chen, Yu; Sun, Haiyi; Liu, Yonghong; Wang, Jingwei; Wang, Cheng; Wang, Tiejun; Li, Ruxin; Xu, Zhizhan; Chin, See Leang

2016-01-01

A unified picture of femtosecond laser induced precipitation in a cloud chamber is proposed. Among the three principal consequences of filamentation from the point of view of thermodynamics, namely, generation of chemicals, shock waves and thermal air flow motion (due to convection), the last one turns out to be the principal cause. Much of the filament induced chemicals would stick onto the existing background CCN’s (Cloud Condensation Nuclei) through collision making the latter more active. Strong mixing of air having a large temperature gradient would result in supersaturation in which the background CCN’s would grow efficiently into water/ice/snow. This conclusion was supported by two independent experiments using pure heating or a fan to imitate the laser-induced thermal effect or the strong air flow motion, respectively. Without the assistance of any shock wave and chemical CCN’s arising from laser filament, condensation and precipitation occurred. Meanwhile we believe that latent heat release during condensation /precipitation would enhance the air flow for mixing. PMID:27143227

Black carbon mixing state impacts on cloud microphysical properties: effects of aerosol plume and environmental conditions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ching, Ping Pui; Riemer, Nicole; West, Matthew

2016-05-27

Black carbon (BC) is usually mixed with other aerosol species within individual aerosol particles. This mixture, along with the particles' size and morphology, determines the particles' optical and cloud condensation nuclei properties, and hence black carbon's climate impacts. In this study the particle-resolved aerosol model PartMC-MOSAIC was used to quantify the importance of black carbon mixing state for predicting cloud microphysical quantities. Based on a set of about 100 cloud parcel simulations a process level analysis framework was developed to attribute the response in cloud microphysical properties to changes in the underlying aerosol population ("plume effect") and the cloud parcelmore » cooling rate ("parcel effect"). It shows that the response of cloud droplet number concentration to changes in BC emissions depends on the BC mixing state. When the aerosol population contains mainly aged BC particles an increase in BC emission results in increasing cloud droplet number concentrations ("additive effect"). In contrast, when the aerosol population contains mainly fresh BC particles they act as sinks for condensable gaseous species, resulting in a decrease in cloud droplet number concentration as BC emissions are increased ("competition effect"). Additionally, we quantified the error in cloud microphysical quantities when neglecting the information on BC mixing state, which is often done in aerosol models. The errors ranged from -12% to +45% for the cloud droplet number fraction, from 0% to +1022% for the nucleation-scavenged black carbon (BC) mass fraction, from -12% to +4% for the effective radius, and from -30% to +60% for the relative dispersion.« less

Impacts of New Particle Formation on Midwestern Climate and Air Quality as Determined by the NPF-explicit WRF-Chem

NASA Astrophysics Data System (ADS)

Dong, C.; Stanier, C. O.; Bullard, R.; Singh, A.

2016-12-01

A one month simulation has been performed using the New particle formation (NPF)-explicit WRF-Chem (Matsui et al, Journal of Geophysical Research, 116(D19208), 2011). The simulation was run for a domain of the continental United States, with analysis focused on the Midwestern and eastern portions of the U.S. Analysis focused on quantification and explanation of planetary boundary layer (PBL) NPF in the model on variables beyond condensation nuclei (CN), cloud condensation nuclei (CCN), and cloud droplet size distributions. The model was evaluated against meteorology, chemical species and aerosol physical property observations. Comparison shows the model performance was comparable to that of other studies. Nucleation enhanced the concentration of condensation nuclei (CN). Cloud condensation nuclei (CCN) concentrations were enhanced and suppressed at high and low supersaturations, respectively. For air pollutants, the most pronounced influence of PBL nucleation was PM2.5 reduction, which was mainly caused by SO4 decreases (62.7%). For shortwave radiation, changes due to indirect effects of NPF were larger than direct effects. Shortwave radiation and cloud droplet concentration typically changed in the same way. Similar change patterns were found for T2 and PBL height. PBL nucleation led to a net increase of precipitation during the simulation period. Sensitivity tests showed that the combination of PBL NPF together with aqueous chemistry was the predominant cause of SO4 reduction.

The Atmospheric Radiation Measurement Program May 2003 Intensive Operations Period Examining Aerosol Properties and Radiative Influences: Preface to Special Section

NASA Technical Reports Server (NTRS)

Ferrare, Richard; Feingold, Graham; Ghan, Steven; Ogren, John; Schmid, Beat; Schwartz, Stephen E.; Sheridan, Pat

2006-01-01

Atmospheric aerosols influence climate by scattering and absorbing radiation in clear air (direct effects) and by serving as cloud condensation nuclei, modifying the microphysical properties of clouds, influencing radiation and precipitation development (indirect effects). Much of present uncertainty in forcing of climate change is due to uncertainty in the relations between aerosol microphysical and optical properties and their radiative influences (direct effects) and between microphysical properties and their ability to serve as cloud condensation nuclei at given supersaturations (indirect effects). This paper introduces a special section that reports on a field campaign conducted at the Department of Energy Atmospheric Radiation Measurement site in North Central Oklahoma in May, 2003, examining these relations using in situ airborne measurements and surface-, airborne-, and space-based remote sensing.

Jets and Water Clouds on Jupiter

NASA Astrophysics Data System (ADS)

Lian, Yuan; Showman, A. P.

2012-10-01

Ground-based and spacecraft observations show that Jupiter exhibits multiple banded zonal jet structures. These banded jets correlate with dark and bright clouds, often called "belts" and "zones". The mechanisms that produce these banded zonal jets and clouds are poorly understood. Our previous studies showed that the latent heat released by condensation of water vapor could produce equatorial superrotation along with multiple zonal jets in the mid-to-high latitudes. However, that previous work assumed complete and instant removal of condensate and therefore could not predict the cloud formation. Here we present an improved 3D Jupiter model to investigate some effects of cloud microphysics on large-scale dynamics using a closed water cycle that includes condensation, three-dimensional advection of cloud material by the large-scale circulation, evaporation and sedimentation. We use a dry convective adjustment scheme to adjust the temperature towards a dry adiabat when atmospheric columns become convectively unstable, and the tracers are mixed within the unstable layers accordingly. Other physics parameterizations included in our model are the bottom drag and internal heat flux as well as the choices of either Newtonian heating scheme or gray radiative transfer. Given the poorly understood cloud microphysics, we perform case studies by treating the particle size and condensation/evaporation time scale as free parameters. We find that, in some cases, the active water cycle can produce multiple banded jets and clouds. However, the equatorial jet is generally very weak in all the cases because of insufficient supply of eastward eddy momentum fluxes. These differences may result from differences in the overall vertical stratification, baroclinicity, and moisture distribution in our new models relative to the older ones; we expect to elucidate the dynamical mechanisms in continuing work.

Cloud Condensation Nuclei Activity of Aerosols during GoAmazon 2014/15 Field Campaign Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, J.; Martin, S. T.; Kleinman, L.

2016-03-01

Aerosol indirect effects, which represent the impact of aerosols on climate through influencing the properties of clouds, remain one of the main uncertainties in climate predictions (Stocker et al. 2013). Reducing this large uncertainty requires both improved understanding and representation of aerosol properties and processes in climate models, including the cloud activation properties of aerosols. The Atmospheric System Research (ASR) science program plan of January 2010 states that: “A key requirement for simulating aerosol-cloud interactions is the ability to calculate cloud condensation nuclei and ice nuclei (CCN and IN, respectively) concentrations as a function of supersaturation from the chemical andmore » microphysical properties of the aerosol.” The Observations and Modeling of the Green Ocean Amazon (GoAmazon 2014/15) study seeks to understand how aerosol and cloud life cycles are influenced by pollutant outflow from a tropical megacity (Manaus)—in particular, the differences in cloud-aerosol-precipitation interactions between polluted and pristine conditions. One key question of GoAmazon2014/5 is: “What is the influence of the Manaus pollution plume on the cloud condensation nuclei (CCN) activities of the aerosol particles and the secondary organic material in the particles?” To address this question, we measured size-resolved CCN spectra, a critical measurement for GoAmazon2014/5.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tan, Xianyu; Showman, Adam P., E-mail: xianyut@lpl.arizona.edu

The growing number of observations of brown dwarfs (BDs) has provided evidence for strong atmospheric circulation on these objects. Directly imaged planets share similar observations and can be viewed as low-gravity versions of BDs. Vigorous condensate cycles of chemical species in their atmospheres are inferred by observations and theoretical studies, and latent heating associated with condensation is expected to be important in shaping atmospheric circulation and influencing cloud patchiness. We present a qualitative description of the mechanisms by which condensational latent heating influences circulation, and then illustrate them using an idealized general circulation model that includes a condensation cycle ofmore » silicates with latent heating and molecular weight effect due to the rainout of the condensate. Simulations with conditions appropriate for typical T dwarfs exhibit the development of localized storms and east–west jets. The storms are spatially inhomogeneous, evolving on a timescale of hours to days and extending vertically from the condensation level to the tropopause. The fractional area of the BD covered by active storms is small. Based on a simple analytic model, we quantitatively explain the area fraction of moist plumes and show its dependence on the radiative timescale and convective available potential energy (CAPE). We predict that if latent heating dominates cloud formation processes, the fractional coverage area of clouds decreases as the spectral type goes through the L/T transition from high to lower effective temperature. This is a natural consequence of the variation of the radiative timescale and CAPE with the spectral type.« less

Clouds in Super-Earth Atmospheres: Chemical Equilibrium Calculations

NASA Astrophysics Data System (ADS)

Mbarek, Rostom; Kempton, Eliza M.-R.

2016-08-01

Recent studies have unequivocally proven the existence of clouds in super-Earth atmospheres. Here we provide a theoretical context for the formation of super-Earth clouds by determining which condensates are likely to form under the assumption of chemical equilibrium. We study super-Earth atmospheres of diverse bulk composition, which are assumed to form by outgassing from a solid core of chondritic material, following Schaefer & Fegley. The super-Earth atmospheres that we study arise from planetary cores made up of individual types of chondritic meteorites. They range from highly reducing to oxidizing and have carbon to oxygen (C:O) ratios that are both sub-solar and super-solar, thereby spanning a range of atmospheric composition that is appropriate for low-mass exoplanets. Given the atomic makeup of these atmospheres, we minimize the global Gibbs free energy of formation for over 550 gases and condensates to obtain the molecular composition of the atmospheres over a temperature range of 350-3000 K. Clouds should form along the temperature-pressure boundaries where the condensed species appear in our calculation. We find that the composition of condensate clouds depends strongly on both the H:O and C:O ratios. For the super-Earth archetype GJ 1214b, KCl and ZnS are the primary cloud-forming condensates at solar composition, in agreement with previous work. However, for oxidizing atmospheres, K2SO4 and ZnO condensates are favored instead, and for carbon-rich atmospheres with super-solar C:O ratios, graphite clouds appear. For even hotter planets, clouds form from a wide variety of rock-forming and metallic species.

CO2 Condensation Models for Mars

NASA Technical Reports Server (NTRS)

Colaprete, A.; Haberle, R.

2004-01-01

During the polar night in both hemispheres of Mars, regions of low thermal emission, frequently referred to as "cold spots", have been observed by Mariner 9, Viking and Mars Global Surveyor (MGS) spacecraft. These cold spots vary in time and appear to be associated with topographic features suggesting that they are the result of a spectral-emission effect due to surface accumulation of fine-grained frost or snow. Presented here are simulations of the Martian polar night using the NASA Ames General Circulation Cloud Model. This cloud model incorporates all the microphysical processes of carbon dioxide cloud formation, including nucleation, condensation and sedimentation and is coupled to a surface frost scheme that includes both direct surface condensation and precipitation. Using this cloud model we simulate the Mars polar nights and compare model results to observations from the Thermal Emission Spectrometer (TES) and the Mars Orbiter Laser Altimeter (MOLA). Model predictions of "cold spots" compare well with TES observations of low emissivity regions, both spatially and as a function of season. The model predicted frequency of CO2 cloud formation also agrees well with MOLA observations of polar night cloud echoes. Together the simulations and observations in the North indicate a distinct shift in atmospheric state centered about Ls 270 which we believe may be associated with the strength of the polar vortex.

Clouds Composition in Super-Earth Atmospheres: Chemical Equilibrium Calculations

NASA Astrophysics Data System (ADS)

Kempton, Eliza M.-R.; Mbarek, Rostom

2015-12-01

Attempts to determine the composition of super-Earth atmospheres have so far been plagued by the presence of clouds. Yet the theoretical framework to understand these clouds is still in its infancy. For the super-Earth archetype GJ 1214b, KCl, Na2S, and ZnS have been proposed as condensates that would form under the condition of chemical equilibrium, if the planet’s atmosphere has a bulk composition near solar. Condensation chemistry calculations have not been presented for a wider range of atmospheric bulk composition that is to be expected for super-Earth exoplanets. Here we provide a theoretical context for the formation of super-Earth clouds in atmospheres of varied composition by determining which condensates are likely to form, under the assumption of chemical equilibrium. We model super-Earth atmospheres assuming they are formed by degassing of volatiles from a solid planetary core of chondritic material. Given the atomic makeup of these atmospheres, we minimize the global Gibbs free energy of over 550 gases and condensates to obtain the molecular composition of the atmospheres over a temperature range of 350-3,000 K. Clouds should form along the temperature-pressure boundaries where the condensed species appear in our calculations. The super-Earth atmospheres that we study range from highly reducing to oxidizing and have carbon to oxygen (C:O) ratios that are both sub-solar and super-solar, thereby spanning a diverse range of atmospheric composition that is appropriate for low-mass exoplanets. Some condensates appear across all of our models. However, the majority of condensed species appear only over specific ranges of H:O and C:O ratios. We find that for GJ 1214b, KCl is the primary cloud-forming condensate at solar composition, in agreement with previous work. However, for oxidizing atmospheres, where H:O is less than unity, K2SO4 clouds form instead. For carbon-rich atmospheres with super-solar C:O ratios, graphite clouds additionally appear. At higher temperatures, clouds are formed from a variety of materials including metals, metal oxides, and aluminosilicates.

Dynamics and thermodynamics of a tornado: Rotation effects

NASA Astrophysics Data System (ADS)

Ben-Amots, N.

2016-09-01

This paper investigates the relevant processes in the tornado including the dynamics of rotation and thermodynamics as well as condensation. The main novelty of this paper is the explanation of the phenomena occurring in the central downflow. The reduced pressure in the tornado's funnel sucks air and water vapor from the cloud above the tornado. The latent heat of condensation is released in the funnel. The centrifugal force drives the generated water drops out of the funnel. The latent heat of condensation released is also transferred out of the funnel, and supplies the helically ascending air flow surrounding the tornado with additional buoyancy energy. This process gives the tornado increased strength compared to the dust devil type of flow, thus explaining why tornadoes occur always under a cloud, and why the tornado pipe can reach a height of a kilometer and more. To sustain a tornado, the temperature of water vapor at the cloud's base should be higher than the surroundings by a certain minimal value. Remote infrared temperature measurements of clouds' bases may provide indications of the probability that a cloud can spawn a tornado, which may increase the lead time.

Cloud Microphysics Budget in the Tropical Deep Convective Regime

NASA Technical Reports Server (NTRS)

Li, Xiao-Fan; Sui, C.-H.; Lau, K.-M.; Einaudi, Franco (Technical Monitor)

2001-01-01

Cloud microphysics budgets in the tropical deep convective regime are analyzed based on a 2-D cloud resolving simulation. The model is forced by the large-scale vertical velocity and zonal wind and large-scale horizontal advections derived from TOGA COARE for a 20-day period. The role of cloud microphysics is first examined by analyzing mass-weighted mean heat budget and column-integrated moisture budget. Hourly budgets show that local changes of mass-weighted mean temperature and column-integrated moisture are mainly determined by the residuals between vertical thermal advection and latent heat of condensation and between vertical moisture advection and condensation respectively. Thus, atmospheric thermodynamics depends on how cloud microphysical processes are parameterized. Cloud microphysics budgets are then analyzed for raining conditions. For cloud-vapor exchange between cloud system and its embedded environment, rainfall and evaporation of raindrop are compensated by the condensation and deposition of supersaturated vapor. Inside the cloud system, the condensation of supersaturated vapor balances conversion from cloud water to raindrop, snow, and graupel through collection and accretion processes. The deposition of supersaturated vapor balances conversion from cloud ice to snow through conversion and riming processes. The conversion and riming of cloud ice and the accretion of cloud water balance conversion from snow to graupel through accretion process. Finally, the collection of cloud water and the melting of graupel increase raindrop to compensate the loss of raindrop due to rainfall and the evaporation of raindrop.

Tight coupling of particle size and composition in atmospheric cloud droplet activation

NASA Astrophysics Data System (ADS)

Topping, D.; McFiggans, G.

2011-09-01

The substantial uncertainty in the indirect effect on radiative forcing in large part arises from the influences of atmospheric aerosol particles on (i) the brightness of clouds, exerting significant shortwave cooling with no appreciable compensation in the longwave, and on (ii) their ability to precipitate, with implications for cloud cover and lifetime. Predicting the ambient conditions at which aerosol particles may become cloud droplets is largely reliant on an equilibrium relationship derived in 1936. However, the theoretical basis of the relationship restricts its application to particles solely comprising involatile compounds and water, whereas a substantial fraction of particles in the real atmosphere will contain potentially thousands of semi-volatile organic compounds in addition to containing semi-volatile inorganic components such as ammonium nitrate. We show that equilibration of atmospherically reasonable concentrations of organic compounds with a growing particle as the ambient humidity increases has larger implications on cloud droplet formation than any other equilibrium compositional dependence, owing to inextricable linkage between the aerosol composition and a particles size under ambient conditions. Whilst previous attempts to account for co-condensation of gases other than water vapour have been restricted to one inorganic condensate, our method demonstrates that accounting for the co-condensation of any number of organic compounds substantially decreases the saturation ratio of water vapour required for droplet activation. This effect is far greater than any other compositional dependence; moreso even than the unphysical effect of surface tension reduction in aqueous organic mixtures, ignoring differences in bulk and surface surfactant concentrations.

Cloud droplet size distribution broadening during diffusional growth: ripening amplified by deactivation and reactivation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yang, Fan; Kollias, Pavlos; Shaw, Raymond A.

Cloud droplet size distributions (CDSDs), which are related to cloud albedo and lifetime, are usually broader in warm clouds than predicted from adiabatic parcel calculations. We investigate a mechanism for the CDSD broadening using a Lagrangian bin-microphysics cloud parcel model that considers the condensational growth of cloud droplets formed on polydisperse, sub-micrometer aerosols in an adiabatic cloud parcel that undergoes vertical oscillations, such as those due to cloud circulations or turbulence. Results show that the CDSD can be broadened during condensational growth as a result of Ostwald ripening amplified by droplet deactivation and reactivation, which is consistent with Korolev (1995).more » The relative roles of the solute effect, curvature effect, deactivation and reactivation on CDSD broadening are investigated. Deactivation of smaller cloud droplets, which is due to the combination of curvature and solute effects in the downdraft region, enhances the growth of larger cloud droplets and thus contributes particles to the larger size end of the CDSD. Droplet reactivation, which occurs in the updraft region, contributes particles to the smaller size end of the CDSD. In addition, we find that growth of the largest cloud droplets strongly depends on the residence time of cloud droplet in the cloud rather than the magnitude of local variability in the supersaturation fluctuation. This is because the environmental saturation ratio is strongly buffered by smaller cloud droplets. Two necessary conditions for this CDSD broadening, which generally occur in the atmosphere, are: (1) droplets form on polydisperse aerosols of varying hygroscopicity and (2) the cloud parcel experiences upwards and downwards motions. Therefore we expect that this mechanism for CDSD broadening is possible in real clouds. Our results also suggest it is important to consider both curvature and solute effects before and after cloud droplet activation in a cloud model. The importance of this mechanism compared with other mechanisms on cloud properties should be investigated through in-situ measurements and 3-D dynamic models.« less

Cloud droplet size distribution broadening during diffusional growth: ripening amplified by deactivation and reactivation

DOE PAGES

Yang, Fan; Kollias, Pavlos; Shaw, Raymond A.; ...

2017-12-06

Cloud droplet size distributions (CDSDs), which are related to cloud albedo and lifetime, are usually broader in warm clouds than predicted from adiabatic parcel calculations. We investigate a mechanism for the CDSD broadening using a Lagrangian bin-microphysics cloud parcel model that considers the condensational growth of cloud droplets formed on polydisperse, sub-micrometer aerosols in an adiabatic cloud parcel that undergoes vertical oscillations, such as those due to cloud circulations or turbulence. Results show that the CDSD can be broadened during condensational growth as a result of Ostwald ripening amplified by droplet deactivation and reactivation, which is consistent with Korolev (1995).more » The relative roles of the solute effect, curvature effect, deactivation and reactivation on CDSD broadening are investigated. Deactivation of smaller cloud droplets, which is due to the combination of curvature and solute effects in the downdraft region, enhances the growth of larger cloud droplets and thus contributes particles to the larger size end of the CDSD. Droplet reactivation, which occurs in the updraft region, contributes particles to the smaller size end of the CDSD. In addition, we find that growth of the largest cloud droplets strongly depends on the residence time of cloud droplet in the cloud rather than the magnitude of local variability in the supersaturation fluctuation. This is because the environmental saturation ratio is strongly buffered by smaller cloud droplets. Two necessary conditions for this CDSD broadening, which generally occur in the atmosphere, are: (1) droplets form on polydisperse aerosols of varying hygroscopicity and (2) the cloud parcel experiences upwards and downwards motions. Therefore we expect that this mechanism for CDSD broadening is possible in real clouds. Our results also suggest it is important to consider both curvature and solute effects before and after cloud droplet activation in a cloud model. The importance of this mechanism compared with other mechanisms on cloud properties should be investigated through in-situ measurements and 3-D dynamic models.« less

Cloud droplet size distribution broadening during diffusional growth: ripening amplified by deactivation and reactivation

NASA Astrophysics Data System (ADS)

Yang, Fan; Kollias, Pavlos; Shaw, Raymond A.; Vogelmann, Andrew M.

2018-05-01

Cloud droplet size distributions (CDSDs), which are related to cloud albedo and rain formation, are usually broader in warm clouds than predicted from adiabatic parcel calculations. We investigate a mechanism for the CDSD broadening using a moving-size-grid cloud parcel model that considers the condensational growth of cloud droplets formed on polydisperse, submicrometer aerosols in an adiabatic cloud parcel that undergoes vertical oscillations, such as those due to cloud circulations or turbulence. Results show that the CDSD can be broadened during condensational growth as a result of Ostwald ripening amplified by droplet deactivation and reactivation, which is consistent with early work. The relative roles of the solute effect, curvature effect, deactivation and reactivation on CDSD broadening are investigated. Deactivation of smaller cloud droplets, which is due to the combination of curvature and solute effects in the downdraft region, enhances the growth of larger cloud droplets and thus contributes particles to the larger size end of the CDSD. Droplet reactivation, which occurs in the updraft region, contributes particles to the smaller size end of the CDSD. In addition, we find that growth of the largest cloud droplets strongly depends on the residence time of cloud droplet in the cloud rather than the magnitude of local variability in the supersaturation fluctuation. This is because the environmental saturation ratio is strongly buffered by numerous smaller cloud droplets. Two necessary conditions for this CDSD broadening, which generally occur in the atmosphere, are as follows: (1) droplets form on aerosols of different sizes, and (2) the cloud parcel experiences upwards and downwards motions. Therefore we expect that this mechanism for CDSD broadening is possible in real clouds. Our results also suggest it is important to consider both curvature and solute effects before and after cloud droplet activation in a cloud model. The importance of this mechanism compared with other mechanisms on cloud properties should be investigated through in situ measurements and 3-D dynamic models.

The observed influence of local anthropogenic pollution on northern Alaskan cloud properties

NASA Astrophysics Data System (ADS)

Maahn, Maximilian; de Boer, Gijs; Creamean, Jessie M.; Feingold, Graham; McFarquhar, Greg M.; Wu, Wei; Mei, Fan

2017-12-01

Due to their importance for the radiation budget, liquid-containing clouds are a key component of the Arctic climate system. Depending on season, they can cool or warm the near-surface air. The radiative properties of these clouds depend strongly on cloud drop sizes, which are governed in part by the availability of cloud condensation nuclei. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska. For this, we use aircraft in situ observations of clouds and aerosols from the 5th Department of Energy Atmospheric Radiation Measurement (DOE ARM) Program's Airborne Carbon Measurements (ACME-V) campaign obtained in summer 2015. Comparison of observations from an area with petroleum extraction facilities (Oliktok Point) with data from a reference area relatively free of anthropogenic sources (Utqiaġvik/Barrow) represents an opportunity to quantify the impact of local industrial emissions on cloud properties. In the presence of local industrial emissions, the mean effective radii of cloud droplets are reduced from 12.2 to 9.4 µm, which leads to suppressed drizzle production and precipitation. At the same time, concentrations of refractory black carbon and condensation nuclei are enhanced below the clouds. These results demonstrate that the effects of anthropogenic pollution on local climate need to be considered when planning Arctic industrial infrastructure in a warming environment.

Broadening of cloud droplet spectra through turbulent entrainment and eddy hopping

NASA Astrophysics Data System (ADS)

Abade, Gustavo; Grabowski, Wojciech; Pawlowska, Hanna

2017-11-01

This work discusses the effect of cloud turbulence and turbulent entrainment on the evolution of the cloud droplet-size spectrum. We simulate an ensemble of idealized turbulent cloud parcels that are subject to entrainment events, modeled as a random Poisson process. Entrainment events, subsequent turbulent mixing inside the parcel, supersaturation fluctuations, and the resulting stochastic droplet growth by condensation are simulated using a Monte Carlo scheme. Quantities characterizing the turbulence intensity, entrainment rate and the mean fraction of environmental air entrained in an event are specified as external parameters. Cloud microphysics is described by applying Lagrangian particles, the so-called superdroplets. They are either unactivated cloud condensation nuclei (CCN) or cloud droplets that form from activated CCN. The model accounts for the transport of environmental CCN into the cloud by the entraining eddies at the cloud edge. Turbulent mixing of the entrained dry air with cloudy air is described using a linear model. We show that turbulence plays an important role in aiding entrained CCN to activate, providing a source of small cloud droplets and thus broadening the droplet size distribution. Further simulation results will be reported at the meeting.

Global Survey of the Relationship Between Cloud Droplet Size and Albedo Using ISCCP

NASA Technical Reports Server (NTRS)

Han, Qingyuan; Rossow, William B.; Chou, Joyce; Welch, Ronald M.

1997-01-01

Aerosols affect climate through direct and indirect effects. The direct effect of aerosols (e.g., sulfates) includes reflection of sunlight back toward space and for some aerosols (e.g., smoke particles), absorption in the atmosphere; both effects cool the Earth's surface. The indirect effect of aerosols refers to the modification of cloud microphysical properties, thereby affecting the radiation balance. Higher concentrations of Cloud Condensation Nuclei (CCN) generally produce higher concentrations of cloud droplets, which are also usually assumed to lead to decreased cloud droplet sizes. The result is an increase in cloud albedo, producing a net radiative cooling, opposite to the warming caused by greenhouse gases (Charlson et al. 1992). The change in clouds that is directly induced by an increase of aerosol concentration is an increase of cloud droplet number density, N; but is is usually assumed that cloud droplet size decreases as if the water mass density Liquid Water Content (LWC) were constant. There is actually no reason why this should be the case. Shifting the cloud droplet size distribution to more numerous smaller droplets can change the relative rates of condensational and coalescence growth, leading to different LWC (e.g., Rossow 1978). Moreover, the resulting change in cloud albedo is usually ascribed to more efficient scattering by smaller droplets, when in fact it is the increase in droplet number density (assuming constant LWC) that produces the most important change in cloud albedo: e.g., holding N constant and decreasing the droplet size would actually decrease the scattering cross-section and, thus, the albedo much more than it is increased by the increased scattering efficiency.

CLOUDS IN SUPER-EARTH ATMOSPHERES: CHEMICAL EQUILIBRIUM CALCULATIONS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mbarek, Rostom; Kempton, Eliza M.-R., E-mail: mbarekro@grinnell.edu, E-mail: kemptone@grinnell.edu

Recent studies have unequivocally proven the existence of clouds in super-Earth atmospheres. Here we provide a theoretical context for the formation of super-Earth clouds by determining which condensates are likely to form under the assumption of chemical equilibrium. We study super-Earth atmospheres of diverse bulk composition, which are assumed to form by outgassing from a solid core of chondritic material, following Schaefer and Fegley. The super-Earth atmospheres that we study arise from planetary cores made up of individual types of chondritic meteorites. They range from highly reducing to oxidizing and have carbon to oxygen (C:O) ratios that are both sub-solarmore » and super-solar, thereby spanning a range of atmospheric composition that is appropriate for low-mass exoplanets. Given the atomic makeup of these atmospheres, we minimize the global Gibbs free energy of formation for over 550 gases and condensates to obtain the molecular composition of the atmospheres over a temperature range of 350–3000 K. Clouds should form along the temperature–pressure boundaries where the condensed species appear in our calculation. We find that the composition of condensate clouds depends strongly on both the H:O and C:O ratios. For the super-Earth archetype GJ 1214b, KCl and ZnS are the primary cloud-forming condensates at solar composition, in agreement with previous work. However, for oxidizing atmospheres, K{sub 2}SO{sub 4} and ZnO condensates are favored instead, and for carbon-rich atmospheres with super-solar C:O ratios, graphite clouds appear. For even hotter planets, clouds form from a wide variety of rock-forming and metallic species.« less

ERTS-1 views the Great Lakes

NASA Technical Reports Server (NTRS)

Lyons, W. A.; Pease, S. R.

1973-01-01

The meteorological content of ERTS images, particularly mesoscale effects of the Great Lakes and air pollution dispersion is summarized. Summertime lake breeze frontal clouds and various winter lake-effect convection patterns and snow squalls are revealed in great detail. A clear-cut spiral vortex over southern Lake Michigan is related to a record early snow storm in the Chicago area. Marked cloud changes induced by orographic and frictional effects on Lake Michigan's lee shore snow squalls are seen. The most important finding, however, is a clear-cut example of alterations in cumulus convection by anthropogenic condensation and/or ice nuclei from northern Indiana steel mills during a snow squall situation. Jet aircraft condensation trails are also found with surprising frequency.

Partially soluble organics as cloud condensation nuclei: Role of trace soluble and surface active species

NASA Astrophysics Data System (ADS)

Broekhuizen, K.; Kumar, P. Pradeep; Abbatt, J. P. D.

2004-01-01

The ability of partially soluble organic species to act as cloud condensation nuclei (CCN) has been studied. A Köhler model incorporating solute solubility and droplet surface tension describes the behavior of solid adipic and succinic acid particles, whereas solid azelaic acid activates much more efficiently that predicted. In addition, it was shown that trace levels of either sulfate or surface active species have a dramatic effect on the activation of adipic acid, a moderately soluble organic, as predicted by the full Köhler model. For internally mixed particles in the atmosphere, these effects will greatly enhance the role of organic aerosols as CCN.

Water Ice Cloud Opacities and Temperatures Derived from the Viking IRTM Data Set

NASA Technical Reports Server (NTRS)

TamppariL. K.; Zurek, R. W.; Paige, D. A.

1999-01-01

The degree to which water ice clouds play a role in the Mars climate is unknown. Latent heating of water ice clouds is small and since most hazes appeared to be thin (tau less than or = 1) their radiative effects have been neglected. Condensation likely limits the vertical extent of water vapor in the water column and a lowering of the condensation altitude, as seen in the northern spring and summer, could increase the seasonal exchange of water between the atmosphere and the surface. It has been suggested that water ice cloud formation is more frequent and widespread in the aphelic hemisphere (currently the northern). This may limit water to the northern hemisphere through greater exchange with the regolith and through restricted southward transport of water vapor by the Mars Hadley circulation. In addition, it has been suggested that water ice cloud formation also controls the vertical distribution of atmospheric dust in some seasons. This scavenging of dust may Continuing from the IRTM cloud maps, derived cloud opacities and cloud temperatures for several locations and seasons will be presented. Sensitivities to cloud particle sizes, surface temperature, and dust opacity will be discussed.

Cloud Condensation in Titan's Lower Stratosphere

NASA Technical Reports Server (NTRS)

Romani, Paul N.; Anderson, Carrie M.

2011-01-01

A 1-D condensation model is developed for the purpose of reproducing ice clouds in Titan's lower stratosphere observed by the Composite Infrared Spectrometer (CIRS) onboard Cassini. Hydrogen cyanide (HCN), cyanoacetylene (HC3N), and ethane (C2H6) vapors are treated as chemically inert gas species that flow from an upper boundary at 500 km to a condensation sink near Titan's tropopause (-45 km). Gas vertical profiles are determined from eddy mixing and a downward flux at the upper boundary. The condensation sink is based upon diffusive growth of the cloud particles and is proportional to the degree of supersaturation in the cloud formation regIOn. Observations of the vapor phase abundances above the condensation levels and the locations and properties of the ice clouds provide constraints on the free parameters in the model. Vapor phase abundances are determined from CIRS mid-IR observations, whereas cloud particle sizes, altitudes, and latitudinal distributions are derived from analyses of CIRS far-IR observations of Titan. Specific cloud constraints include: I) mean particle radii of2-3 J.lm inferred from the V6 506 cm- band of HC3N, 2) latitudinal abundance distributions of condensed nitriles, inferred from a composite emission feature that peaks at 160/cm , and 3) a possible hydrocarbon cloud layer at high latitudes, located near an altitude of 60 km, which peaks between 60 and 80 cm l . Nitrile abundances appear to diminish substantially at high northern latitudes over the time period 2005 to 2010 (northern mid winter to early spring). Use of multiple gas species provides a consistency check on the eddy mixing coefficient profile. The flux at the upper boundary is the net column chemical production from the upper atmosphere and provides a constraint on chemical pathways leading to the production of these compounds. Comparison of the differing lifetimes, vapor phase transport, vapor phase loss rate, and particle sedimentation, sheds light on temporal stability of the clouds.

Ship Tracks

Atmospheric Science Data Center

2013-04-19

... into a moist layer of atmosphere. The particles become cloud condensation nuclei (CCN), which may either produce new cloud particles where ... visualization of the vertical structure of the condensation trails. It was created using a combination of red band data from ...

Attribution of the United States “warming hole”: Aerosol indirect effect andprecipitable water vapor

EPA Science Inventory

Aerosols can influence the climate indirectly by acting as cloud condensation nuclei and /or ice nuclei, thereby modifying cloud optical properties. Observations show a striking cooling trend in summertime daily maximum temperature (T_max) in the central and...

Organic condensation: a vital link connecting aerosol formation to cloud condensation nuclei (CCN) concentrations

NASA Astrophysics Data System (ADS)

Riipinen, I.; Pierce, J. R.; Yli-Juuti, T.; Nieminen, T.; Häkkinen, S.; Ehn, M.; Junninen, H.; Lehtipalo, K.; Petäjä, T.; Slowik, J.; Chang, R.; Shantz, N. C.; Abbatt, J.; Leaitch, W. R.; Kerminen, V.-M.; Worsnop, D. R.; Pandis, S. N.; Donahue, N. M.; Kulmala, M.

2011-04-01

Atmospheric aerosol particles influence global climate as well as impair air quality through their effects on atmospheric visibility and human health. Ultrafine (<100 nm) particles often dominate aerosol numbers, and nucleation of atmospheric vapors is an important source of these particles. To have climatic relevance, however, the freshly nucleated particles need to grow in size. We combine observations from two continental sites (Egbert, Canada and Hyytiälä, Finland) to show that condensation of organic vapors is a crucial factor governing the lifetimes and climatic importance of the smallest atmospheric particles. We model the observed ultrafine aerosol growth with a simplified scheme approximating the condensing species as a mixture of effectively non-volatile and semi-volatile species, demonstrate that state-of-the-art organic gas-particle partitioning models fail to reproduce the observations, and propose a modeling approach that is consistent with the measurements. We find that roughly half of the mass of the condensing mass needs to be distributed proportional to the aerosol surface area (thus implying that the condensation is governed by gas-phase concentration rather than the equilibrium vapour pressure) to explain the observed aerosol growth. We demonstrate the large sensitivity of predicted number concentrations of cloud condensation nuclei (CCN) to these interactions between organic vapors and the smallest atmospheric nanoparticles - highlighting the need for representing this process in global climate models.

Aerosol effect on cloud droplet size as monitored from surface-based remote sensing over East China Sea region

NASA Astrophysics Data System (ADS)

Pandithurai, G.; Takamura, T.; Yamaguchi, J.; Miyagi, K.; Takano, T.; Ishizaka, Y.; Dipu, S.; Shimizu, A.

2009-07-01

The effect of increased aerosol concentrations on the low-level, non-precipitating, ice-free stratus clouds is examined using a suite of surface-based remote sensing systems. Cloud droplet effective radius and liquid water path are retrieved using cloud radar and microwave radiometer. Collocated measurements of aerosol scattering coefficient, size distribution and cloud condensation nuclei (CCN) concentrations were used to examine the response of cloud droplet size and optical thickness to increased CCN proxies. During the episodic events of increase in aerosol accumulation-mode volume distribution, the decrease in droplet size and increase in cloud optical thickness is observed. The indirect effect estimates are made for both droplet effective radius and cloud optical thickness for different liquid water path ranges and they range 0.02-0.18 and 0.005-0.154, respectively. Data are also categorized into thin and thick clouds based on cloud geometric thickness (Δz) and estimates show IE values are relatively higher for thicker clouds.

Laser-filamentation-induced condensation and snow formation in a cloud chamber.

PubMed

Ju, Jingjing; Liu, Jiansheng; Wang, Cheng; Sun, Haiyi; Wang, Wentao; Ge, Xiaochun; Li, Chuang; Chin, See Leang; Li, Ruxin; Xu, Zhizhan

2012-04-01

Using 1 kHz, 9 mJ femtosecond laser pulses, we demonstrate laser-filamentation-induced spectacular snow formation in a cloud chamber. An intense updraft of warm moist air is generated owing to the continuous heating by the high-repetition filamentation. As it encounters the cold air above, water condensation and large-sized particles spread unevenly across the whole cloud chamber via convection and cyclone like action on a macroscopic scale. This indicates that high-repetition filamentation plays a significant role in macroscopic laser-induced water condensation and snow formation.

The observed influence of local anthropogenic pollution on northern Alaskan cloud properties

DOE Office of Scientific and Technical Information (OSTI.GOV)

Maahn, Maximilian; de Boer, Gijs; Creamean, Jessie M.

Due to their importance for the radiation budget, liquid-containing clouds are a key component of the Arctic climate system. Depending on season, they can cool or warm the near-surface air. The radiative properties of these clouds depend strongly on cloud drop sizes, which are governed in part by the availability of cloud condensation nuclei. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska. For this, we use aircraft in situ observations of clouds and aerosols from the 5th Department of Energy Atmospheric Radiation Measurement (DOE ARM)more » Program's Airborne Carbon Measurements (ACME-V) campaign obtained in summer 2015. Comparison of observations from an area with petroleum extraction facilities (Oliktok Point) with data from a reference area relatively free of anthropogenic sources (Utqiaġvik/Barrow) represents an opportunity to quantify the impact of local industrial emissions on cloud properties. In the presence of local industrial emissions, the mean effective radii of cloud droplets are reduced from 12.2 to 9.4 µm, which leads to suppressed drizzle production and precipitation. At the same time, concentrations of refractory black carbon and condensation nuclei are enhanced below the clouds. These results demonstrate that the effects of anthropogenic pollution on local climate need to be considered when planning Arctic industrial infrastructure in a warming environment.« less

The observed influence of local anthropogenic pollution on northern Alaskan cloud properties

DOE Office of Scientific and Technical Information (OSTI.GOV)

Maahn, Maximilian; de Boer, Gijs; Creamean, Jessie M.

Due to their importance for the radiation budget, liquid-containing clouds are a key component of the Arctic climate system. Depending on season, they can cool or warm the near-surface air. The radiative properties of these clouds depend strongly on cloud drop sizes, which are governed in part by the availability of cloud condensation nuclei. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska. For this, we use aircraft in situ observations of clouds and aerosols from the 5th Department of Energy Atmospheric Radiation Measurement (DOE ARM)more » Program's Airborne Carbon Measurements (ACME-V) campaign obtained in summer 2015. Comparison of observations from an area with petroleum extraction facilities (Oliktok Point) with data from a reference area relatively free of anthropogenic sources (Utqiagvik/Barrow) represents an opportunity to quantify the impact of local industrial emissions on cloud properties. In the presence of local industrial emissions, the mean effective radii of cloud droplets are reduced from 12.2 to 9.4 µm, which leads to suppressed drizzle production and precipitation. At the same time, concentrations of refractory black carbon and condensation nuclei are enhanced below the clouds. These results demonstrate that the effects of anthropogenic pollution on local climate need to be considered when planning Arctic industrial infrastructure in a warming environment.« less

The observed influence of local anthropogenic pollution on northern Alaskan cloud properties

DOE PAGES

Maahn, Maximilian; de Boer, Gijs; Creamean, Jessie M.; ...

2017-12-11

Due to their importance for the radiation budget, liquid-containing clouds are a key component of the Arctic climate system. Depending on season, they can cool or warm the near-surface air. The radiative properties of these clouds depend strongly on cloud drop sizes, which are governed in part by the availability of cloud condensation nuclei. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska. For this, we use aircraft in situ observations of clouds and aerosols from the 5th Department of Energy Atmospheric Radiation Measurement (DOE ARM)more » Program's Airborne Carbon Measurements (ACME-V) campaign obtained in summer 2015. Comparison of observations from an area with petroleum extraction facilities (Oliktok Point) with data from a reference area relatively free of anthropogenic sources (Utqiagvik/Barrow) represents an opportunity to quantify the impact of local industrial emissions on cloud properties. In the presence of local industrial emissions, the mean effective radii of cloud droplets are reduced from 12.2 to 9.4 µm, which leads to suppressed drizzle production and precipitation. At the same time, concentrations of refractory black carbon and condensation nuclei are enhanced below the clouds. These results demonstrate that the effects of anthropogenic pollution on local climate need to be considered when planning Arctic industrial infrastructure in a warming environment.« less

The Impacts of an Observationally-Based Cloud Fraction and Condensate Overlap Parameterization on a GCM's Cloud Radiative Effect

NASA Technical Reports Server (NTRS)

Oreopoulos, Lazaros; Lee, Dongmin; Norris, Peter; Yuan, Tianle

2011-01-01

It has been shown that the details of how cloud fraction overlap is treated in GCMs has substantial impact on shortwave and longwave fluxes. Because cloud condensate is also horizontally heterogeneous at GCM grid scales, another aspect of cloud overlap should in principle also be assessed, namely the vertical overlap of hydrometeor distributions. This type of overlap is usually examined in terms of rank correlations, i.e., linear correlations between hydrometeor amount ranks of the overlapping parts of cloud layers at specific separation distances. The cloud fraction overlap parameter and the rank correlation of hydrometeor amounts can be both expressed as inverse exponential functions of separation distance characterized by their respective decorrelation lengths (e-folding distances). Larger decorrelation lengths mean that hydrometeor fractions and probability distribution functions have high levels of vertical alignment. An analysis of CloudSat and CALIPSO data reveals that the two aspects of cloud overlap are related and their respective decorrelation lengths have a distinct dependence on latitude that can be parameterized and included in a GCM. In our presentation we will contrast the Cloud Radiative Effect (CRE) of the GEOS-5 atmospheric GCM (AGCM) when the observationally-based parameterization of decorrelation lengths is used to represent overlap versus the simpler cases of maximum-random overlap and globally constant decorrelation lengths. The effects of specific overlap representations will be examined for both diagnostic and interactive radiation runs in GEOS-5 and comparisons will be made with observed CREs from CERES and CloudSat (2B-FLXHR product). Since the radiative effects of overlap depend on the cloud property distributions of the AGCM, the availability of two different cloud schemes in GEOS-5 will give us the opportunity to assess a wide range of potential cloud overlap consequences on the model's climate.

Microphysical Processes Affecting the Pinatubo Volcanic Plume

NASA Technical Reports Server (NTRS)

Hamill, Patrick; Houben, Howard; Young, Richard; Turco, Richard; Zhao, Jingxia

1996-01-01

In this paper we consider microphysical processes which affect the formation of sulfate particles and their size distribution in a dispersing cloud. A model for the dispersion of the Mt. Pinatubo volcanic cloud is described. We then consider a single point in the dispersing cloud and study the effects of nucleation, condensation and coagulation on the time evolution of the particle size distribution at that point.

Biogenic influence on cloud microphysics in the 'clean' oceanic atmosphere

NASA Astrophysics Data System (ADS)

Lana, A.; Simó, R.; Vallina, S. M.; Jurado, E.; Dachs, J.

2009-12-01

A 20 years old hypothesis postulates a feedback relationship between marine biota and climate through the emission of dimethylsulfide (DMS) as the principal natural source of Sulfate Secondary Aerosols (S-DMS) that are very efficient as cloud condensation nuclei (CCN). In recent years, the biological influence on cloud microphysics have been expanded to other potential biogenic cloud precursors: (i) volatile organic compounds produced by plankton and emitted to the atmosphere to form Secondary Organic Aerosols (SOA); (ii) biological particles and biogenic polymers, lifted with the seaspray by wind friction and bubble-bursting processes, that act as Primary Organic Aerosols (POA). Besides these biogenic aerosols, also seaspray-associated Sea Salt (SS) emissions, which are the dominant contribution to aerosol mass in the remote mixed boundary layer, also contribute to cloud condensation. All these aerosols affect cloud microphysics by providing new CCN, reducing the size of cloud droplets, and increasing cloud albedo. We have compared the seasonalities of the parameterized source functions of these natural cloud precursors with that of the satellite-derived cloud droplet effective radius (CLEFRA) over large regions of the ocean. Regions where big loads of continental aerosols (including anthropogenic -industrial, urban, and biomass burning) dominate during a significant part of the year were identified by use of remote sensing aerosol optical properties and excluded from our analysis. Our results show that the seasonality of cloud droplet effective radius matches those of S-DMS and SOA in the clean marine atmosphere, whereas SS and chlorophyll-associated POA on their own do not seem to play a major role in driving cloud droplet size.

Reducing Errors in Satellite Simulated Views of Clouds with an Improved Parameterization of Unresolved Scales

NASA Astrophysics Data System (ADS)

Hillman, B. R.; Marchand, R.; Ackerman, T. P.

2016-12-01

Satellite instrument simulators have emerged as a means to reduce errors in model evaluation by producing simulated or psuedo-retrievals from model fields, which account for limitations in the satellite retrieval process. Because of the mismatch in resolved scales between satellite retrievals and large-scale models, model cloud fields must first be downscaled to scales consistent with satellite retrievals. This downscaling is analogous to that required for model radiative transfer calculations. The assumption is often made in both model radiative transfer codes and satellite simulators that the unresolved clouds follow maximum-random overlap with horizontally homogeneous cloud condensate amounts. We examine errors in simulated MISR and CloudSat retrievals that arise due to these assumptions by applying the MISR and CloudSat simulators to cloud resolving model (CRM) output generated by the Super-parameterized Community Atmosphere Model (SP-CAM). Errors are quantified by comparing simulated retrievals performed directly on the CRM fields with those simulated by first averaging the CRM fields to approximately 2-degree resolution, applying a "subcolumn generator" to regenerate psuedo-resolved cloud and precipitation condensate fields, and then applying the MISR and CloudSat simulators on the regenerated condensate fields. We show that errors due to both assumptions of maximum-random overlap and homogeneous condensate are significant (relative to uncertainties in the observations and other simulator limitations). The treatment of precipitation is particularly problematic for CloudSat-simulated radar reflectivity. We introduce an improved subcolumn generator for use with the simulators, and show that these errors can be greatly reduced by replacing the maximum-random overlap assumption with the more realistic generalized overlap and incorporating a simple parameterization of subgrid-scale cloud and precipitation condensate heterogeneity. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. SAND NO. SAND2016-7485 A

Precipitating Condensation Clouds in Substellar Atmospheres

NASA Technical Reports Server (NTRS)

Ackerman, Andrew S.; Marley, Mark S.; Gore, Warren J. (Technical Monitor)

2000-01-01

We present a method to calculate vertical profiles of particle size distributions in condensation clouds of giant planets and brown dwarfs. The method assumes a balance between turbulent diffusion and precipitation in horizontally uniform cloud decks. Calculations for the Jovian ammonia cloud are compared with previous methods. An adjustable parameter describing the efficiency of precipitation allows the new model to span the range of predictions from previous models. Calculations for the Jovian ammonia cloud are found to be consistent with observational constraints. Example calculations are provided for water, silicate, and iron clouds on brown dwarfs and on a cool extrasolar giant planet.

From aerosol-limited to invigoration of warm convective clouds.

PubMed

Koren, Ilan; Dagan, Guy; Altaratz, Orit

2014-06-06

Among all cloud-aerosol interactions, the invigoration effect is the most elusive. Most of the studies that do suggest this effect link it to deep convective clouds with a warm base and cold top. Here, we provide evidence from observations and numerical modeling of a dramatic aerosol effect on warm clouds. We propose that convective-cloud invigoration by aerosols can be viewed as an extension of the concept of aerosol-limited clouds, where cloud development is limited by the availability of cloud-condensation nuclei. A transition from pristine to slightly polluted atmosphere yields estimated negative forcing of ~15 watts per square meter (cooling), suggesting that a substantial part of this anthropogenic forcing over the oceans occurred at the beginning of the industrial era, when the marine atmosphere experienced such transformation. Copyright © 2014, American Association for the Advancement of Science.

Worldwide data sets constrain the water vapor uptake coefficient in cloud formation

PubMed Central

Raatikainen, Tomi; Nenes, Athanasios; Seinfeld, John H.; Morales, Ricardo; Moore, Richard H.; Lathem, Terry L.; Lance, Sara; Padró, Luz T.; Lin, Jack J.; Cerully, Kate M.; Bougiatioti, Aikaterini; Cozic, Julie; Ruehl, Christopher R.; Chuang, Patrick Y.; Anderson, Bruce E.; Flagan, Richard C.; Jonsson, Haflidi; Mihalopoulos, Nikos; Smith, James N.

2013-01-01

Cloud droplet formation depends on the condensation of water vapor on ambient aerosols, the rate of which is strongly affected by the kinetics of water uptake as expressed by the condensation (or mass accommodation) coefficient, αc. Estimates of αc for droplet growth from activation of ambient particles vary considerably and represent a critical source of uncertainty in estimates of global cloud droplet distributions and the aerosol indirect forcing of climate. We present an analysis of 10 globally relevant data sets of cloud condensation nuclei to constrain the value of αc for ambient aerosol. We find that rapid activation kinetics (αc > 0.1) is uniformly prevalent. This finding resolves a long-standing issue in cloud physics, as the uncertainty in water vapor accommodation on droplets is considerably less than previously thought. PMID:23431189

Worldwide data sets constrain the water vapor uptake coefficient in cloud formation.

PubMed

Raatikainen, Tomi; Nenes, Athanasios; Seinfeld, John H; Morales, Ricardo; Moore, Richard H; Lathem, Terry L; Lance, Sara; Padró, Luz T; Lin, Jack J; Cerully, Kate M; Bougiatioti, Aikaterini; Cozic, Julie; Ruehl, Christopher R; Chuang, Patrick Y; Anderson, Bruce E; Flagan, Richard C; Jonsson, Haflidi; Mihalopoulos, Nikos; Smith, James N

2013-03-05

Cloud droplet formation depends on the condensation of water vapor on ambient aerosols, the rate of which is strongly affected by the kinetics of water uptake as expressed by the condensation (or mass accommodation) coefficient, αc. Estimates of αc for droplet growth from activation of ambient particles vary considerably and represent a critical source of uncertainty in estimates of global cloud droplet distributions and the aerosol indirect forcing of climate. We present an analysis of 10 globally relevant data sets of cloud condensation nuclei to constrain the value of αc for ambient aerosol. We find that rapid activation kinetics (αc > 0.1) is uniformly prevalent. This finding resolves a long-standing issue in cloud physics, as the uncertainty in water vapor accommodation on droplets is considerably less than previously thought.

Influence of organic films on the evaporation and condensation of water in aerosol

PubMed Central

Davies, James F.; Miles, Rachael E. H.; Haddrell, Allen E.; Reid, Jonathan P.

2013-01-01

Uncertainties in quantifying the kinetics of evaporation and condensation of water from atmospheric aerosol are a significant contributor to the uncertainty in predicting cloud droplet number and the indirect effect of aerosols on climate. The influence of aerosol particle surface composition, particularly the impact of surface active organic films, on the condensation and evaporation coefficients remains ambiguous. Here, we report measurements of the influence of organic films on the evaporation and condensation of water from aerosol particles. Significant reductions in the evaporation coefficient are shown to result when condensed films are formed by monolayers of long-chain alcohols [CnH(2n+1)OH], with the value decreasing from 2.4 × 10−3 to 1.7 × 10−5 as n increases from 12 to 17. Temperature-dependent measurements confirm that a condensed film of long-range order must be formed to suppress the evaporation coefficient below 0.05. The condensation of water on a droplet coated in a condensed film is shown to be fast, with strong coherence of the long-chain alcohol molecules leading to islanding as the water droplet grows, opening up broad areas of uncoated surface on which water can condense rapidly. We conclude that multicomponent composition of organic films on the surface of atmospheric aerosol particles is likely to preclude the formation of condensed films and that the kinetics of water condensation during the activation of aerosol to form cloud droplets is likely to remain rapid. PMID:23674675

Influence of organic films on the evaporation and condensation of water in aerosol.

PubMed

Davies, James F; Miles, Rachael E H; Haddrell, Allen E; Reid, Jonathan P

2013-05-28

Uncertainties in quantifying the kinetics of evaporation and condensation of water from atmospheric aerosol are a significant contributor to the uncertainty in predicting cloud droplet number and the indirect effect of aerosols on climate. The influence of aerosol particle surface composition, particularly the impact of surface active organic films, on the condensation and evaporation coefficients remains ambiguous. Here, we report measurements of the influence of organic films on the evaporation and condensation of water from aerosol particles. Significant reductions in the evaporation coefficient are shown to result when condensed films are formed by monolayers of long-chain alcohols [C(n)H(2n+1)OH], with the value decreasing from 2.4 × 10(-3) to 1.7 × 10(-5) as n increases from 12 to 17. Temperature-dependent measurements confirm that a condensed film of long-range order must be formed to suppress the evaporation coefficient below 0.05. The condensation of water on a droplet coated in a condensed film is shown to be fast, with strong coherence of the long-chain alcohol molecules leading to islanding as the water droplet grows, opening up broad areas of uncoated surface on which water can condense rapidly. We conclude that multicomponent composition of organic films on the surface of atmospheric aerosol particles is likely to preclude the formation of condensed films and that the kinetics of water condensation during the activation of aerosol to form cloud droplets is likely to remain rapid.

Integrating Cloud Processes in the Community Atmosphere Model, Version 5.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Park, S.; Bretherton, Christopher S.; Rasch, Philip J.

2014-09-15

This paper provides a description on the parameterizations of global cloud system in CAM5. Compared to the previous versions, CAM5 cloud parameterization has the following unique characteristics: (1) a transparent cloud macrophysical structure that has horizontally non-overlapped deep cumulus, shallow cumulus and stratus in each grid layer, each of which has own cloud fraction, mass and number concentrations of cloud liquid droplets and ice crystals, (2) stratus-radiation-turbulence interaction that allows CAM5 to simulate marine stratocumulus solely from grid-mean RH without relying on the stability-based empirical empty stratus, (3) prognostic treatment of the number concentrations of stratus liquid droplets and icemore » crystals with activated aerosols and detrained in-cumulus condensates as the main sources and evaporation-sedimentation-precipitation of stratus condensate as the main sinks, and (4) radiatively active cumulus. By imposing consistency between diagnosed stratus fraction and prognosed stratus condensate, CAM5 is free from empty or highly-dense stratus at the end of stratus macrophysics. CAM5 also prognoses mass and number concentrations of various aerosol species. Thanks to the aerosol activation and the parameterizations of the radiation and stratiform precipitation production as a function of the droplet size, CAM5 simulates various aerosol indirect effects associated with stratus as well as direct effects, i.e., aerosol controls both the radiative and hydrological budgets. Detailed analysis of various simulations revealed that CAM5 is much better than CAM3/4 in the global performance as well as the physical formulation. However, several problems were also identifed, which can be attributed to inappropriate regional tuning, inconsistency between various physics parameterizations, and incomplete model physics. Continuous efforts are going on to further improve CAM5.« less

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

NASA Technical Reports Server (NTRS)

Zamora, L. M.; Kahn, R. A.; Cubison, M. J.; Diskin, G. S.; Jimenez, J. L.; Kondo, Y.; McFarquhar, G. M.; Nenes, A.; Thornhill, K. L.; Wisthaler, A.;

Aircraft-measured indirect cloud effects from biomass burning smoke in the Arctic and subarctic

DOE PAGES

Zamora, Lauren M.; Kahn, R. A.; Cubison, M. J.; ...

2016-01-21

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200–300% over the next 50–100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were ~40–60% smallermore » than in background clouds. Based on the relationship between cloud droplet number ( N liq) and various biomass burning tracers (BB t) across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol–cloud interactions (ACIs, where ACI = (1/3) × d ln( N liq)/d ln(BB t)) to be ~0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (~0.02gm –3) and very high aerosol concentrations (2000–3000 cm –3) in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 Wm –2 or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic. Furthermore, we lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.« less

Physical and Optical/Radiative Characteristics of Aerosol and Cloud Particles in Tropical Cirrus: Importance in Radiation Balance

NASA Technical Reports Server (NTRS)

Pueschel, R. F.; Howard, S. D.; Foster, T. C.; Hallett, J.; Arnott, W. P.; Condon, Estelle P. (Technical Monitor)

1996-01-01

Whether cirrus clouds heat or cool the Earth-atmosphere system depends on the relative importance of the cloud shortwave albedo effect and the cloud thermal greenhouse effect. Both are determined by the distribution of ice condensate with cloud particle size. The microphysics instrument package flown aboard the NASA DC-8 in TOGA/COARE included an ice crystal replicator, a 2D Greyscale Cloud Particle Probe and a Forward Scattering Spectrometer Aerosol Probe. In combination, the electro-optical instruments permitted particle size measurements between 0.5 micrometer and 2.6 millimeter diameter. Ice crystal replicas were used to validate signals from the electrooptical instruments. Both optical and scanning electron microscopy were utilized to analyze aerosol and ice particle replicas between 0.1 micrometer and several 100 micrometer diameter. In first approximation, the combined aerosol-cloud particle spectrum in several clouds followed a power law N alpha D(sup -2.5). Thus, large cloud particles carried most of the condensate mass, while small cloud and aerosol particles determined the surface area. The mechanism of formation of small particles is growth of (hygroscopic, possibly ocean-derived) aerosol particles along the Kohler curves. The concentration of small particles is higher and less variable in space and time, and their tropospheric residence time is longer, than those of large cloud particles because of lower sedimentation velocities. Small particles shift effective cloud particle radii to sizes much smaller than the mean diameter of the cloud particles. This causes an increase in shortwave reflectivity and IR emissivity, and a decrease in transmissivity. Occasionally, the cloud reflectivity increased with altitude (decreasing temperature) stronger than did cloud emissivity, yielding enhanced radiative cooling at higher altitudes. Thus, cirrus produced by deep convection in the tropics may be critical in controlling processes whereby energy from warm tropical oceans is injected to different levels in the atmosphere to subsequently influence not only tropical but mid-latitude climate.

A study of cloud microphysics and precipitation over the Tibetan Plateau by radar observations and cloud-resolving model simulations: Cloud Microphysics over Tibetan Plateau

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gao, Wenhua; Sui, Chung-Hsiung; Fan, Jiwen

Cloud microphysical properties and precipitation over the Tibetan Plateau (TP) are unique because of the high terrains, clean atmosphere, and sufficient water vapor. With dual-polarization precipitation radar and cloud radar measurements during the Third Tibetan Plateau Atmospheric Scientific Experiment (TIPEX-III), the simulated microphysics and precipitation by the Weather Research and Forecasting model (WRF) with the Chinese Academy of Meteorological Sciences (CAMS) microphysics and other microphysical schemes are investigated through a typical plateau rainfall event on 22 July 2014. Results show that the WRF-CAMS simulation reasonably reproduces the spatial distribution of 24-h accumulated precipitation, but has limitations in simulating time evolutionmore » of precipitation rates. The model-calculated polarimetric radar variables have biases as well, suggesting bias in modeled hydrometeor types. The raindrop sizes in convective region are larger than those in stratiform region indicated by the small intercept of raindrop size distribution in the former. The sensitivity experiments show that precipitation processes are sensitive to the changes of warm rain processes in condensation and nucleated droplet size (but less sensitive to evaporation process). Increasing droplet condensation produces the best area-averaged rain rate during weak convection period compared with the observation, suggesting a considerable bias in thermodynamics in the baseline simulation. Increasing the initial cloud droplet size causes the rain rate reduced by half, an opposite effect to that of increasing droplet condensation.« less

Height Dependency of Aerosol-Cloud Interaction Regimes: Height Dependency of ACI Regime

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chen, Jingyi; Liu, Yangang; Zhang, Minghua

This study investigates the height dependency of aerosol-cloud interaction regimes in terms of the joint dependence of the key cloud microphysical properties (e.g. cloud droplet number concentration, cloud droplet relative dispersion, etc.) on aerosol number concentration (N a) and vertical velocity (w). The three distinct regimes with different microphysical features are the aerosol-limited regime, the updraft-limited regime, and the transitional regime. The results reveal two new phenomena in updraft-limited regime: 1) The “condensational broadening” of cloud droplet size distribution in contrast to the well-known “condensational narrowing” in the aerosol-limited regime; 2) Above the level of maximum supersaturation, some cloud dropletsmore » are deactivated into interstitial aerosols in the updraft-limited regime whereas all droplets remain activated in the aerosol-limited regime. Further analysis shows that the particle equilibrium supersaturation plays important role in understanding these unique features. Also examined is the height of warm rain initiation and its dependence on N a and w. The rain initiation height is found to depend primarily on either N a or w or both in different N a-w regimes, thus suggesting a strong regime dependence of the second aerosol indirect effect.« less

Height Dependency of Aerosol-Cloud Interaction Regimes: Height Dependency of ACI Regime

DOE PAGES

Chen, Jingyi; Liu, Yangang; Zhang, Minghua; ...

2018-01-10

This study investigates the height dependency of aerosol-cloud interaction regimes in terms of the joint dependence of the key cloud microphysical properties (e.g. cloud droplet number concentration, cloud droplet relative dispersion, etc.) on aerosol number concentration (N a) and vertical velocity (w). The three distinct regimes with different microphysical features are the aerosol-limited regime, the updraft-limited regime, and the transitional regime. The results reveal two new phenomena in updraft-limited regime: 1) The “condensational broadening” of cloud droplet size distribution in contrast to the well-known “condensational narrowing” in the aerosol-limited regime; 2) Above the level of maximum supersaturation, some cloud dropletsmore » are deactivated into interstitial aerosols in the updraft-limited regime whereas all droplets remain activated in the aerosol-limited regime. Further analysis shows that the particle equilibrium supersaturation plays important role in understanding these unique features. Also examined is the height of warm rain initiation and its dependence on N a and w. The rain initiation height is found to depend primarily on either N a or w or both in different N a-w regimes, thus suggesting a strong regime dependence of the second aerosol indirect effect.« less

Aircraft profile measurements of 18O/16O and D/H isotope ratios of cloud condensate and water vapor constrain precipitation efficiency and entrainment rates in tropical clouds

NASA Astrophysics Data System (ADS)

Noone, D. C.; Raudzens Bailey, A.; Toohey, D. W.; Twohy, C. H.; Heymsfield, A.; Rella, C.; Van Pelt, A. D.

2011-12-01

Convective clouds play a significant role in the moisture and heat balance of the tropics. The dynamics of organized and isolated convection are a function of the background thermodynamic profile and wind shear, buoyancy sources near the surface and the latent heating inside convective updrafts. The stable oxygen and hydrogen isotope ratios in water vapor and condensate can be used to identify dominant moisture exchanges and aspects of the cloud microphysics that are otherwise difficult to observe. Both the precipitation efficiency and the dilution of cloud updrafts by entrainment can be estimated since the isotopic composition outside the plume is distinct from inside. Measurements of the 18O/16O and D/H isotope ratios were made in July 2011 on 13 research flights of the NCAR C130 aircraft during the ICE-T (Ice in Clouds Experiment - Tropical) field campaign near St Croix. Measurements were made using an instrument based on the Picarro Wave-Length Scanning Cavity Ring Down platform that includes a number of optical, hardware and software modifications to allow measurements to be made at 5 Hz for deployment on aircraft. The measurement system was optimized to make precise measurements of the isotope ratio of liquid and ice cloud condensate by coupling the gas analyzer to the NCAR Counter flow Virtual Impactor inlet. The inlet system provides a particle enhancement while rejecting vapor. Sample air is vigorously heated before flowing into the gas phase analyzer. We present statistics that demonstrate the performance and calibration of the instrument. Measured profiles show that environmental air exhibits significant layering showing controls from boundary layer processes, large scale horizontal advection and regional subsidence. Condensate in clouds is consistent with generally low precipitation efficiency, although there is significant variability in the isotope ratios suggesting heterogeneity within plumes and the stochastic nature of detrainment processes. Entrainment of air into the plume is seen as evaporation of condensate. In the plume between about -7 and -12C, the ice condensate fraction increases with height, and the isotope ratios are used to discern ice formation from deposition from ice formed from in situ freezing of cloud liquid. The observed profiles demonstrate a new capacity for cloud process studies and provide new insight into the water budget of clouds.

Stratus Cloud Radiative Effects from Cloud Processed Bimodal CCN Distributions

NASA Astrophysics Data System (ADS)

Noble, S. R., Jr.; Hudson, J. G.

2016-12-01

Inability to understand cloud processes is a large component of climate uncertainty. Increases in cloud condensation nuclei (CCN) concentrations are known to increase cloud droplet number concentrations (Nc). This aerosol-cloud interaction (ACI) produces greater Nc at smaller sizes, which brightens clouds. A lesser understood ACI is cloud processing of CCN. This improves CCN that then more easily activate at lower cloud supersaturations (S). Bimodal CCN distributions thus ensue from these evaporated cloud droplets. Hudson et al. (2015) related CCN bimodality to Nc. In stratus clouds, bimodal CCN created greater Nc whereas in cumulus less Nc. Thus, CCN distribution shape influences cloud properties; microphysics and radiative properties. Measured uni- and bimodal CCN distributions were input into an adiabatic droplet growth model using various specified vertical wind speeds (W). Bimodal CCN produced greater Nc (Fig. 1a) and smaller mean diameters (MD; Fig. 1b) at lower W typical of stratus clouds (<70 cm/s). Improved CCN (low critical S) were more easily activated at the lower S of stratus from low W, thus, creating greater Nc. Competition for condensate thus reduced MD and drizzle. At greater W, typical of cumulus clouds (>70 cm/s), bimodal CCN made lower Nc with larger MD thus enhancing drizzle whereas unimodal CCN made greater Nc with smaller MD, thus reducing drizzle. Thus, theoretical predictions of Nc and MD for uni- and bimodal CCN agree with the sense of the observations. Radiative effects were determined using a cloud grown to a 250-meter thickness. Bimodal CCN at low W reduced cloud effective radius (re), made greater cloud optical thickness (COT), and made greater cloud albedo (Fig. 1c). At very low W changes were as much as +9% for albedo, +17% for COT, and -12% for re. Stratus clouds typically have low W and cover large areas. Thus, these changes in cloud radiative properties at low W impact climate. Stratus cloud susceptibility to CCN distribution thus requires further investigation to determine their impact on ACI. Hudson et al. (2015), JGRA, 120, 3436-3452.

A Fast and Efficient Version of the TwO-Moment Aerosol Sectional (TOMAS) Global Aerosol Microphysics Model

NASA Technical Reports Server (NTRS)

Lee, Yunha; Adams, P. J.

2012-01-01

This study develops more computationally efficient versions of the TwO-Moment Aerosol Sectional (TOMAS) microphysics algorithms, collectively called Fast TOMAS. Several methods for speeding up the algorithm were attempted, but only reducing the number of size sections was adopted. Fast TOMAS models, coupled to the GISS GCM II-prime, require a new coagulation algorithm with less restrictive size resolution assumptions but only minor changes in other processes. Fast TOMAS models have been evaluated in a box model against analytical solutions of coagulation and condensation and in a 3-D model against the original TOMAS (TOMAS-30) model. Condensation and coagulation in the Fast TOMAS models agree well with the analytical solution but show slightly more bias than the TOMAS-30 box model. In the 3-D model, errors resulting from decreased size resolution in each process (i.e., emissions, cloud processing wet deposition, microphysics) are quantified in a series of model sensitivity simulations. Errors resulting from lower size resolution in condensation and coagulation, defined as the microphysics error, affect number and mass concentrations by only a few percent. The microphysics error in CN70CN100 (number concentrations of particles larger than 70100 nm diameter), proxies for cloud condensation nuclei, range from 5 to 5 in most regions. The largest errors are associated with decreasing the size resolution in the cloud processing wet deposition calculations, defined as cloud-processing error, and range from 20 to 15 in most regions for CN70CN100 concentrations. Overall, the Fast TOMAS models increase the computational speed by 2 to 3 times with only small numerical errors stemming from condensation and coagulation calculations when compared to TOMAS-30. The faster versions of the TOMAS model allow for the longer, multi-year simulations required to assess aerosol effects on cloud lifetime and precipitation.

The global impact of mineral dust on cloud droplet number concentration

NASA Astrophysics Data System (ADS)

Karydis, V.; Tsimpidi, A.; Bacer, S.; Pozzer, A.; Nenes, A.; Lelieveld, J.

2016-12-01

This study assesses the importance of mineral dust for cloud droplet formation by taking into account i) the adsorption of water on the surface of insoluble dust particles, ii) the coating of soluble material on the surface of mineral particles which augments their cloud condensation nuclei activity, and iii) the effect of dust on the inorganic aerosol concentrations through thermodynamic interactions with mineral cations. Simulations are carried out with the EMAC chemistry climate model that calculates the global atmospheric aerosol composition using the ISORROPIA-II thermodynamic equilibrium model and considers the gas phase interactions with K+-Ca2+-Mg2+-NH4+-Na+-SO42-NO3-Cl-H2O particle components. Emissions of the inert mineral dust and the reactive dust aerosol components are calculated online by taking into account the soil particle size distribution and chemical composition of different deserts worldwide (Karydis et al., 2016). We have implemented the "unified dust activation parameterization" (Kumar et al., 2011; Karydis et al., 2011) to calculate the droplet number concentration by taking into account the inherent hydrophilicity from adsorption and the acquired hygroscopicity from soluble salts by dust particles. Our simulations suggest that mineral dust significantly increases the cloud droplet number concentration (CDNC) over the main deserts and the adjacent oceans. However, over polluted areas the CDNC decreases significantly in the presence of dust. Furthermore, we investigate the role of adsorption activation of insoluble aerosols and the mineral dust thermodynamic interactions with inorganic anions on the cloud droplet formation. The CDNC sensitivity to the emission load, chemical composition, and inherent hydrophilicity of mineral dust is also tested. ReferencesKarydis, et al. (2011). "On the effect of dust particles on global cloud condensation nuclei and cloud droplet number." J. Geophys. Res. Atmos. 116. Karydis, et al. (2016). "Effects of mineral dust on global atmospheric nitrate concentrations." Atmos. Chem. Phys. 16(3): 1491-1509. Kumar, et al. (2011). "Measurements of cloud condensation nuclei activity and droplet activation kinetics of wet processed regional dust samples and minerals." Atmos. Chem. Phys. Discuss. 11(4): 12561-12605.

A Review of Spatial and Seasonal Changes in Condensation Clouds Observed During Aerobraking by MGS TES

NASA Technical Reports Server (NTRS)

Pearl, J. C.; Smith, M. D.; Conrath, B. J.; Bandfield, J. L.; Christensen, P. R.

1999-01-01

Successful operation of the Mars Global Surveyor spacecraft beginning in September 1997, has permitted extensive infrared observations of condensation clouds during the martian southern summer and fall seasons (184 deg

Electroscavenging and Inferred Effects on Precipitation Efficiency

NASA Astrophysics Data System (ADS)

Tinsley, B. A.

2002-12-01

The evaporation of charged droplets leaves charged aerosol particles that can act as cloud condensation nuclei and ice forming nuclei. New calculations of scavenging of such charged particles by droplets have been made, that now include the effects of inertia and variable particle density, and variable cloud altitudes ranging into the stratosphere. They show that the Greenfield Gap closes for particles of low density, or for high altitude clouds, or for a few hundred elementary charges on the particles. A few tens of elementary charges on the particles gives collision efficiencies typically an order of magnitude greater than that due to phoretic forces alone. The numerical integrations show that electroscavenging of ice forming nuclei leading to contact ice nucleation is competitive with deposition ice nucleation, for cloud top temperatures in the range 0§C to -15§C and droplet size distributions extending past 10-15 mm radius. This implies that for marine stratocumulus or nimbostratus clouds with tops just below freezing temperature, where precipitation is initiated by the Wegener-Bergeron-Findeisen process, the precipitation efficiency can be affected by the amount of charge on the ice-forming nuclei. This in turn depends on the extent of the (weak) electrification of the cloud. Similarly, electroscavenging of condensation nuclei can increase the average droplet size in successive cycles of cloud evaporation and formation, and can also affect precipitation efficiency.

The Third International Cloud Condensation Nuclei Workshop. [conference

NASA Technical Reports Server (NTRS)

Kocmond, W. C.; Rogers, C. R. (Editor); Rea, S. W. (Editor)

1981-01-01

Twenty-five instruments were tested, including size characterization devices and two Aitken counters. The test aerosols were supplied to the instruments by an on-line generation system, thereby eliminating the need for storage bags. Cloud condensation chambers and haze chambers are highlighted.

Effect of ship-stack effluents on cloud reflectivity

NASA Technical Reports Server (NTRS)

Coakley, James A., Jr.; Bernstein, Robert L.; Durkee, Philip A.

1987-01-01

Under stable meteorological conditions the effect of ship-stack exhaust on overlying clouds was detected in daytime satellite images as an enhancement in cloud reflectivity at 3.7 micrometers. The exhaust is a source of cloud-condensation nuclei that increases the number of cloud droplets while reducing droplet size. This reduction in droplet size causes the reflectivity at 3.7 micrometers to be greater than the levels for nearby noncontaminated clouds of similar physical characteristics. The increase in droplet number causes the reflectivity at 0.63 micrometer to be significantly higher for the contaminated clouds despite the likelihood that the exhaust is a source of particles that absorb at visible wavelengths. The effect of aerosols on cloud reflectivity is expected to have a larger influence on the earth's albedo than that due to the direct scattering and absorption of sunlight by the aerosols alone.

HCl in rocket exhaust clouds - Atmospheric dispersion, acid aerosol characteristics, and acid rain deposition

NASA Technical Reports Server (NTRS)

Pellett, G. L.; Sebacher, D. I.; Bendura, R. J.; Wornom, D. E.

1983-01-01

Both measurements and model calculations of the temporal dispersion of peak HCl (g + aq) concentration in Titan III exhaust clouds are found to be well characterized by one-term power-law decay expressions. The respective coefficients and decay exponents, however, are found to vary widely with meteorology. The HCl (g), HCl (g + aq), dewpoint, and temperature-pressure-altitude data for Titan III exhaust clouds are consistent with accurately calculated HCl/H2O vapor-liquid compositions for a model quasi-equilibrated flat surface aqueous aerosol. Some cloud evolution characteristics are also defined. Rapid and extensive condensation of aqueous acid clearly occurs during the first three min of cloud rise. Condensation is found to be intensified by the initial entrainment of relatively moist ambient air from lower levels, that is, from levels below eventual cloud stabilization. It is pointed out that if subsequent dilution air at stabilization altitude is significantly drier, a state of maximum condensation soon occurs, followed by an aerosol evaporation phase.

Remote sensing of smoke, clouds, and fire using AVIRIS data

NASA Technical Reports Server (NTRS)

Gao, Bo-Cai; Kaufman, Yorman J.; Green, Robert O.

1993-01-01

Clouds remain the greatest element of uncertainty in predicting global climate change. During deforestation and biomass burning processes, a variety of atmospheric gases, including CO2 and SO2, and smoke particles are released into the atmosphere. The smoke particles can have important effects on the formation of clouds because of the increased concentration of cloud condensation nuclei. They can also affect cloud albedo through changes in cloud microphysical properties. Recently, great interest has arisen in understanding the interaction between smoke particles and clouds. We describe our studies of smoke, clouds, and fire using the high spatial and spectral resolution data acquired with the NASA/JPL Airborne Visible/Infrared Imaging Spectrometer (AVIRIS).

Macroscopic impacts of cloud and precipitation processes on maritime shallow convection as simulated by a large eddy simulation model with bin microphysics

DOE PAGES

Grabowski, W. W.; Wang, L. -P.; Prabha, T. V.

2015-01-27

This paper discusses impacts of cloud and precipitation processes on macrophysical properties of shallow convective clouds as simulated by a large eddy model applying warm-rain bin microphysics. Simulations with and without collision–coalescence are considered with cloud condensation nuclei (CCN) concentrations of 30, 60, 120, and 240 mg -1. Simulations with collision–coalescence include either the standard gravitational collision kernel or a novel kernel that includes enhancements due to the small-scale cloud turbulence. Simulations with droplet collisions were discussed in Wyszogrodzki et al. (2013) focusing on the impact of the turbulent collision kernel. The current paper expands that analysis and puts modelmore » results in the context of previous studies. Despite a significant increase of the drizzle/rain with the decrease of CCN concentration, enhanced by the effects of the small-scale turbulence, impacts on the macroscopic cloud field characteristics are relatively minor. Model results show a systematic shift in the cloud-top height distributions, with an increasing contribution of deeper clouds for stronger precipitating cases. We show that this is consistent with the explanation suggested in Wyszogrodzki et al. (2013); namely, the increase of drizzle/rain leads to a more efficient condensate offloading in the upper parts of the cloud field. A second effect involves suppression of the cloud droplet evaporation near cloud edges in low-CCN simulations, as documented in previous studies (e.g., Xue and Feingold, 2006). We pose the question whether the effects of cloud turbulence on drizzle/rain formation in shallow cumuli can be corroborated by remote sensing observations, for instance, from space. Although a clear signal is extracted from model results, we argue that the answer is negative due to uncertainties caused by the temporal variability of the shallow convective cloud field, sampling and spatial resolution of the satellite data, and overall accuracy of remote sensing retrievals.« less

STORMVEX. Ice Nuclei and Cloud Condensation Nuclei Characterization Field Campaign Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cziczo, D.

2016-03-01

The relationship between aerosol particles and the formation of clouds is among the most uncertain aspects in our current understanding of climate change. Warm clouds have been the most extensively studied, in large part because they are normally close to the Earth’s surface and only contain large concentrations of liquid droplets. Ice and mixed-phase clouds have been less studied even though they have extensive global coverage and dominate precipitation formation. Because they require low temperatures to form, both cloud types are infrequently found at ground level, resulting in more difficult field studies. Complex mixtures of liquid and ice elements, normallymore » at much lower concentrations than found in warm clouds, require precise separation techniques and accurate identification of phase. Because they have proved so difficult to study, the climatic impact of ice-containing clouds remains unresolved. In this study, cloud condensation nuclei (CCN) concentrations and associated single particles’ composition and size were measured at a high-elevation research site—Storm Peak Lab, east of Steamboat Springs, Colorado, operated by the Desert Research Institute. Detailed composition analyses were presented to compare CCN activation with single-particle composition. In collaboration with the scientists of the Storm Peak Lab Cloud Property Validation Experiment (STORMVEX), our goal was to relate these findings to the cloud characteristics and the effect of anthropogenic activities.« less

Discovery of lake-effect clouds on Titan

USGS Publications Warehouse

Brown, M.E.; Schaller, E.L.; Roe, H.G.; Chen, C.; Roberts, J.; Brown, R.H.; Baines, K.H.; Clark, R.N.

2009-01-01

Images from instruments on Cassini as well as from telescopes on the ground reveal the presence of sporadic small-scale cloud activity in the cold late-winter north polar region of Saturn's large moon Titan. These clouds lie underneath the previously discovered uniform polar cloud attributed to a quiescent ethane cloud at ???40 km and appear confined to the same latitudes as those of the largest known hydrocarbon lakes at the north pole of Titan. The physical properties of these clouds suggest that they are due to methane convection and condensation. Such convection could be caused by a process in some ways analogous to terrestrial lake-effect clouds. The lakes on Titan could be a key connection between the surface and the meteorological cycle. ?? 2009 by the American Geophysical Union.

Wave-Modulated CO2 Condensation in Mars' Polar Atmosphere From MGS/TES & MOLA and MRO/MCS.

NASA Astrophysics Data System (ADS)

Banfield, D. J.

2016-12-01

In Mars' polar night, atmospheric temperatures fall low enough to cause CO2 condensation. This has been empirically demonstrated by Mars Global Surveyor's (MGS) Mars Orbiter Laser Altimeter (MOLA), which identified reflections from above the surface, and MGS Radio Science (RS) and Thermal Emission Spectrometer (TES) and Mars Reconnaissance Orbiter's (MRO) Mars Climate Sounder (MCS), all of which showed polar night temperature profiles that were super-saturated. Detailed analysis of TES temperature profiles as well as numerical modeling both suggest that the stationary and traveling waves on the polar vortices are strong enough to significantly modulate the CO2 cloud condensation. However the extent to which this is actually occurring has not been quantified. The polar night CO2 condensation represents a significant amount of energy deposition, even if it were uniformly distributed. If instead it is concentrated in the cold sectors of the various waves, this can be a tremendous perturbation not only to the wave amplitudes (clipping them from going much below the CO2 condensation temperature), but also impacting their ability to transport heat and momentum poleward and upward, and thus it may also impact the maintenance and shape of the polar vortex itself. Mars' polar vortices remain barotropically unstable throughout the winter in spite of large amplitude waves in their vicinity. We have identified when and where the various waves (with their specific amplitudes and phases) in the vicinity of the polar vortex should modulate the CO2 condensation (see Figure of a meridional cross-section showing where no clouds are expected (blue), clouds should be ubiquitous (green) and waves should be required to form clouds (red)). We have also correlated this with the distribution of the actual observed cloud identifications from MGS MOLA and MRO MCS. We find only poor correlations between the MGS/TES identified wave modulated condensation predictions and actual simultaneous cloud identifications from MGS/MOLA. We will discuss the results of a similar study using only MRO/MCS to analyze the mean atmospheric temperature, the stationary and traveling waves along the polar vortex, and the actual locations where CO2 condensation is evident.

Process-model Simulations of Cloud Albedo Enhancement by Aerosols in the Arctic

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kravitz, Benjamin S.; Wang, Hailong; Rasch, Philip J.

2014-11-17

A cloud-resolving model is used to simulate the effectiveness of Arctic marine cloud brightening via injection of cloud condensation nuclei (CCN). An updated cloud microphysical scheme is employed, with prognostic CCN and cloud particle numbers in both liquid and mixed-phase marine low clouds. Injection of CCN into the marine boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. Because nearly all of the albedo effects are in the liquid phase due to the removal of ice water by snowfall when ice processes are involved, albedo increases are stronger for pure liquid clouds than mixed-phase clouds.more » Liquid precipitation can be suppressed by CCN injection, whereas ice precipitation (snow) is affected less; thus the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. CCN injection into a clean regime results in a greater albedo increase than injection into a polluted regime, consistent with current knowledge about aerosol-cloud interactions. Unlike previous studies investigating warm clouds, dynamical changes in circulation due to precipitation changes are small.« less

The chemical evolution of molecular clouds

NASA Technical Reports Server (NTRS)

Iglesias, E.

1977-01-01

The nonequilibrium chemistry of dense molecular clouds (10,000 to 1 million hydrogen molecules per cu cm) is studied in the framework of a model that includes the latest published chemical data and most of the recent theoretical advances. In this model the only important external source of ionization is assumed to be high-energy cosmic-ray bombardment; standard charge-transfer reactions are taken into account as well as reactions that transfer charge from molecular ions to trace-metal atoms. Schemes are proposed for the synthesis of such species as NCO, HNCO, and CN. The role played by adsorption and condensation of molecules on the surface of dust grains is investigated, and effects on the chemical evolution of a dense molecular cloud are considered which result from varying the total density or the elemental abundances and from assuming negligible or severe condensation of gaseous species on dust grains. It is shown that the chemical-equilibrium time scale is given approximately by the depletion times of oxygen and nitrogen when the condensation efficiency is negligible; that this time scale is probably in the range from 1 to 4 million years, depending on the elemental composition and initial conditions in the cloud; and that this time scale is insensitive to variations in the total density.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zamora, Lauren M.; Kahn, R. A.; Cubison, M. J.

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200–300% over the next 50–100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were ~40–60% smallermore » than in background clouds. Based on the relationship between cloud droplet number ( N liq) and various biomass burning tracers (BB t) across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol–cloud interactions (ACIs, where ACI = (1/3) × d ln( N liq)/d ln(BB t)) to be ~0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (~0.02gm –3) and very high aerosol concentrations (2000–3000 cm –3) in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 Wm –2 or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic. Furthermore, we lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.« less

Cloud Condensation Nuclei Particle Counter (CCN) Instrument Handbook

DOE Office of Scientific and Technical Information (OSTI.GOV)

Uin, Janek

2016-04-01

The Cloud Condensation Nuclei Counter—CCN (Figure 1) is a U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility instrument for measuring the concentration of aerosol particles that can act as cloud condensation nuclei [1, 2]. The CCN draws the sample aerosol through a column with thermodynamically unstable supersaturated water vapor that can condense onto aerosol particles. Particles that are activated, i.e., grown larger in this process, are counted (and sized) by an Optical Particle Counter (OPC). Thus, activated ambient aerosol particle number concentration as a function of supersaturation is measured. Models CCN-100 and CCN-200 differ only inmore » the number of humidifier columns and related subsystems: CCN-100 has one column and CCN-200 has two columns along with dual flow systems and electronics.« less

A Review of Spatial and Seasonal Changes in Condensation Clouds Observed During Aerobraking by MGS TES

NASA Technical Reports Server (NTRS)

Pearl, J. C.; Smith, M. D.; Conrath, B. J.; Bandfield, J. L.; Christensen, P. R.

1999-01-01

Successful operation of the Mars Global Surveyor spacecraft, beginning in September 1997, has permitted extensive infrared observations of condensation clouds during the martian southern summer and fall seasons (184 deg less than L(sub s) less than 28 deg). Initially, thin (normal optical depth less than 0.06 at 825/ cm) ice clouds and hazes were widespread, showing a latitudinal gradient. With the onset of a regional dust storm at L(sub s) = 224 deg, ice clouds essentially vanished in the southern hemisphere, to reappear gradually after the decay of the storm. The thickest clouds (optical depth approx. 0.6) were associated with major volcanic features. At L(exp s) = 318 deg, the cloud at Ascraeus Mons was observed to disappear between 21:30 and 09:30, consistent with historically recorded diurnal behavior for clouds of this type. Limb observations showed extended optically thin (depth less than 0.04) stratiform clouds at altitudes up to 55 km. A water ice haze was present in the north polar night at altitudes up to 40 km; this probably provided heterogeneous nucleation sites for the formation of CO2 clouds at altitudes below the 1 mbar pressure level, where atmospheric temperatures dropped to the condensation point of CO2.

Light in condensed matter in the upper atmosphere as the origin of homochirality: circularly polarized light from Rydberg matter.

PubMed

Holmlid, Leif

2009-01-01

Clouds of the condensed excited Rydberg matter (RM) exist in the atmospheres of comets and planetary bodies (most easily observed at Mercury and the Moon), where they surround the entire bodies. Vast such clouds are recently proposed to exist in the upper atmosphere of Earth (giving rise to the enormous features called noctilucent clouds, polar mesospheric clouds, and polar mesospheric summer radar echoes). It has been shown in experiments with RM that linearly polarized visible light scattered from an RM layer is transformed to circularly polarized light with a probability of approximately 50%. The circular Rydberg electrons in the magnetic field in the RM may be chiral scatterers. The magnetic and anisotropic RM medium acts as a circular polarizer probably by delaying one of the perpendicular components of the light wave. The delay process involved is called Rabi-flopping and gives delays of the order of femtoseconds. This strong effect thus gives intense circularly polarized visible and UV light within RM clouds. Amino acids and other chiral molecules will experience a strong interaction with this light field in the upper atmospheres of planets. The interaction will vary with the stereogenic conformation of the molecules and in all probability promote the survival of one enantiomer. Here, this strong effect is proposed to be the origin of homochirality. The formation of amino acids in the RM clouds is probably facilitated by the catalytic effect of RM.

Light in Condensed Matter in the Upper Atmosphere as the Origin of Homochirality: Circularly Polarized Light from Rydberg Matter

NASA Astrophysics Data System (ADS)

Holmlid, Leif

2009-08-01

Clouds of the condensed excited Rydberg matter (RM) exist in the atmospheres of comets and planetary bodies (most easily observed at Mercury and the Moon), where they surround the entire bodies. Vast such clouds are recently proposed to exist in the upper atmosphere of Earth (giving rise to the enormous features called noctilucent clouds, polar mesospheric clouds, and polar mesospheric summer radar echoes). It has been shown in experiments with RM that linearly polarized visible light scattered from an RM layer is transformed to circularly polarized light with a probability of approximately 50%. The circular Rydberg electrons in the magnetic field in the RM may be chiral scatterers. The magnetic and anisotropic RM medium acts as a circular polarizer probably by delaying one of the perpendicular components of the light wave. The delay process involved is called Rabi-flopping and gives delays of the order of femtoseconds. This strong effect thus gives intense circularly polarized visible and UV light within RM clouds. Amino acids and other chiral molecules will experience a strong interaction with this light field in the upper atmospheres of planets. The interaction will vary with the stereogenic conformation of the molecules and in all probability promote the survival of one enantiomer. Here, this strong effect is proposed to be the origin of homochirality. The formation of amino acids in the RM clouds is probably facilitated by the catalytic effect of RM.

Planetary astronomy

NASA Technical Reports Server (NTRS)

1976-01-01

Color and spectral data from spectrometer observations and computerized analyses of asteroid spectra are discussed. Potential occultations of bright asteroids by the moon are summarized. Analysis of anisotropic scattering within Saturn's rings indicates that mineral contamination of the 120 particles cannot exceed 5 percent by weight, and that the rings formed from particle breakup rather than from particle condensation. Raman probe applications to Jupiter and Uranus atmospheres indicate the presence of aerosol particles. A review of Mariner 9 Mars cloud topography data establishes that most blue clouds are orographic uplift clouds composed of condensates, and that sporadic red clouds are associated with blue clouds or volcanoes and thus probably do not represent dust storm phenomena.

Laser-filamentation-induced water condensation and snow formation in a cloud chamber filled with different ambient gases.

PubMed

Liu, Yonghong; Sun, Haiyi; Liu, Jiansheng; Liang, Hong; Ju, Jingjing; Wang, Tiejun; Tian, Ye; Wang, Cheng; Liu, Yi; Chin, See Leang; Li, Ruxin

2016-04-04

We investigated femtosecond laser-filamentation-induced airflow, water condensation and snow formation in a cloud chamber filled respectively with air, argon and helium. The mass of snow induced by laser filaments was found being the maximum when the chamber was filled with argon, followed by air and being the minimum with helium. We also discussed the mechanisms of water condensation in different gases. The results show that filaments with higher laser absorption efficiency, which result in higher plasma density, are beneficial for triggering intense airflow and thus more water condensation and precipitation.

Determination of Large-Scale Cloud Ice Water Concentration by Combining Surface Radar and Satellite Data in Support of ARM SCM Activities

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Guosheng

2013-03-15

Single-column modeling (SCM) is one of the key elements of Atmospheric Radiation Measurement (ARM) research initiatives for the development and testing of various physical parameterizations to be used in general circulation models (GCMs). The data required for use with an SCM include observed vertical profiles of temperature, water vapor, and condensed water, as well as the large-scale vertical motion and tendencies of temperature, water vapor, and condensed water due to horizontal advection. Surface-based measurements operated at ARM sites and upper-air sounding networks supply most of the required variables for model inputs, but do not provide the horizontal advection term ofmore » condensed water. Since surface cloud radar and microwave radiometer observations at ARM sites are single-point measurements, they can provide the amount of condensed water at the location of observation sites, but not a horizontal distribution of condensed water contents. Consequently, observational data for the large-scale advection tendencies of condensed water have not been available to the ARM cloud modeling community based on surface observations alone. This lack of advection data of water condensate could cause large uncertainties in SCM simulations. Additionally, to evaluate GCMs cloud physical parameterization, we need to compare GCM results with observed cloud water amounts over a scale that is large enough to be comparable to what a GCM grid represents. To this end, the point-measurements at ARM surface sites are again not adequate. Therefore, cloud water observations over a large area are needed. The main goal of this project is to retrieve ice water contents over an area of 10 x 10 deg. surrounding the ARM sites by combining surface and satellite observations. Built on the progress made during previous ARM research, we have conducted the retrievals of 3-dimensional ice water content by combining surface radar/radiometer and satellite measurements, and have produced 3-D cloud ice water contents in support of cloud modeling activities. The approach of the study is to expand a (surface) point measurement to an (satellite) area measurement. That is, the study takes the advantage of the high quality cloud measurements (particularly cloud radar and microwave radiometer measurements) at the point of the ARM sites. We use the cloud ice water characteristics derived from the point measurement to guide/constrain a satellite retrieval algorithm, then use the satellite algorithm to derive the 3-D cloud ice water distributions within an 10° (latitude) x 10° (longitude) area. During the research period, we have developed, validated and improved our cloud ice water retrievals, and have produced and archived at ARM website as a PI-product of the 3-D cloud ice water contents using combined satellite high-frequency microwave and surface radar observations for SGP March 2000 IOP and TWP-ICE 2006 IOP over 10 deg. x 10 deg. area centered at ARM SGP central facility and Darwin sites. We have also worked on validation of the 3-D ice water product by CloudSat data, synergy with visible/infrared cloud ice water retrievals for better results at low ice water conditions, and created a long-term (several years) of ice water climatology in 10 x 10 deg. area of ARM SGP and TWP sites and then compared it with GCMs.« less

Titan's Aerosol and Condensation Cloud Properties in the Far-IR Between 2005 and 2010

NASA Technical Reports Server (NTRS)

Anderson, Carrie; Samuelson, Robert

2011-01-01

Analyses of far-IR spectra between 20 and 560 cm(exp -1) (500 to 18 micron) recorded by the Cassini Composite Infrared Spectrometer (CIRS) yield the spectral dependence and the vertical distribution of Titan's photochemical aerosol and ice clouds. Titan's aerosol appears to be well mixed between the surface and an altitude of 300 km, with a spectral shape that does not change with latitude or time. The aerosol exhibits an extremely broad emission feature with a spectral peak at 140 cm(exp -1) (71 micron), which is not evident in laboratory simulated Titan aerosols (tholin). This low- energy aerosol emission feature may arise from low-energy molecules such as polycyclic aromatic hydrocarbons and/or nitrogenated aromatics. Unlike the vertically well-mixed aerosol, Titan's condensate clouds are located in highly restricted altitudes in the lower stratosphere, ranging between 60 and 100 km at low and moderate latitudes, to between 150 and 165 km at high northern latitudes during northern winter. Such clouds are located at altitudes where nitrile vapors are expected to condense and appear to be dominated by HCN and HC3N, which are the two most abundant nitriles in Titan's atmosphere. Associated with this ice cloud is a broad emission feature that spectrally peaks near 160 cm(exp -1) (62.5 micron). This ice composite appears to chemically change with altitude and latitude, probably as a result of differences in vapor abundance and condensation temperature, and the ice cloud appears to be global in extent. Both CIRS and the Huygens Descent Imager and Spectral Radiometer (DISR) show evidence of cloud layering in Titan's lower stratosphere. The 15 km difference in cloud altitude indicated by the two instruments suggests a difference in ice composition. CIRS also indicates a second ice cloud that exists at isolated latitudes and is consistent with hydrocarbon condensation above the tropopause. This cloud exhibits an emission feature that spectrally peaks near 80 cm(exp -1) (125 micron), possibly due to C2H6 ice or dominated by an ethane-acetylene composite ice, given that CzH6 then C2H2 are the two most abundant hydrocarbons next to methane in Titan's atmosphere.

The Effect of Carbon Dioxide (CO 2) Ice Cloud Condensation on the Habitable Zone

NASA Astrophysics Data System (ADS)

Lincowski, Andrew; Meadows, Victoria; Robinson, Tyler D.; Crisp, David

2016-10-01

The currently accepted outer limit of the habitable zone (OHZ) is defined by the "maximum greenhouse" limit, where Rayleigh scattering from additional CO2 gas overwhelms greenhouse warming. However, this long-standing definition neglects the radiative effects of CO2 clouds (Kopparapu, 2013); this omission was justified based on studies using the two-stream approximation, which found CO2 clouds to be highly likely to produce a net warming. However, recent comparisons of the radiative effect of CO2 clouds using both a two-stream and multi-stream radiative transfer model (Kitzmann et al, 2013; Kitzmann, 2016) found that the warming effect was reduced when the more sophisticated multi-stream models were used. In many cases CO2 clouds caused a cooling effect, meaning that their impact on climate could not be neglected when calculating the outer edge of the habitable zone. To better understand the impact of CO2 ice clouds on the OHZ, we have integrated CO2 cloud condensation into a versatile 1-D climate model for terrestrial planets (Robinson et al, 2012) that uses the validated multi-stream SMART radiative transfer code (Meadows & Crisp, 1996; Crisp, 1997) with a simple microphysical model. We present preliminary results on the habitable zone with self-consistent CO2 clouds for a range of atmospheric masses, compositions and host star spectra, and the subsequent effect on surface temperature. In particular, we evaluate the habitable zone for TRAPPIST-1d (Gillon et al, 2016) with a variety of atmospheric compositions and masses. We present reflectance and transit spectra of these cold terrestrial planets. We identify any consequences for the OHZ in general and TRAPPIST-1d in particular. This more comprehensive treatment of the OHZ could impact our understanding of the distribution of habitable planets in the universe, and provide better constraints for statistical target selection techniques, such as the habitability index (Barnes et al, 2015), for missions like JWST, WFIRST-AFTA and the LUVOIR mission concept.

On signatures of clouds in exoplanetary transit spectra

NASA Astrophysics Data System (ADS)

Pinhas, Arazi; Madhusudhan, Nikku

2017-11-01

Transmission spectra of exoplanetary atmospheres have been used to infer the presence of clouds/hazes. Such inferences are typically based on spectral slopes in the optical deviant from gaseous Rayleigh scattering or low-amplitude spectral features in the infrared. We investigate three observable metrics that could allow constraints on cloud properties from transmission spectra, namely the optical slope, the uniformity of this slope and condensate features in the infrared. We derive these metrics using model transmission spectra considering Mie extinction from a wide range of condensate species, particle sizes and scaleheights. First, we investigate possible degeneracies among the cloud properties for an observed slope. We find, for example, that spectra with very steep optical slopes suggest sulphide clouds (e.g. MnS, ZnS, Na2S) in the atmospheres. Secondly, (non)uniformities in optical slopes provide additional constraints on cloud properties, e.g. MnS, ZnS, TiO2 and Fe2O3 have significantly non-uniform slopes. Thirdly, infrared spectra provide an additional powerful probe into cloud properties, with SiO2, Fe2O3, Mg2SiO4 and MgSiO3 bearing strong infrared features observable with James Webb Space Telescope. We investigate observed spectra of eight hot Jupiters and discuss their implications. In particular, no single or composite condensate species considered here conforms to the steep and non-uniform optical slope observed for HD 189733b. Our work highlights the importance of the three above metrics to investigate cloud properties in exoplanetary atmospheres using high-precision transmission spectra and detailed cloud models. We make our Mie scattering data for condensates publicly available to the community.

Microphysical Model Studies of Venus Clouds

NASA Astrophysics Data System (ADS)

Meade, P. E.; Bullock, M. A.; Grinspoon, D. H.

2004-11-01

We have adapted a standard cloud microphysics model to construct a self-consistent microphysical model of Venus' cloud layer which reproduces and extends previous studies (e.g. James et al. 1997). Our model is based on the Community Aerosol and Radiation Model Atmosphere (CARMA), which is a widely used computer code for terrestrial cloud microphysics, derived from the work of Toon et al. (1988). The standard code has been adapted to treat H2O and H2SO4 as co-condensing vapor species onto aqueous H2SO4 cloud droplets, as well as the nucleation of condensation nuclei to droplets. Vapor condensation and evaporation follows the method of James et al. (1997). Microphysical processes included in this model include nucleation of condensation nuclei, condensation and evaporation of H2O and H2SO4 vapor, and droplet coagulation. Vertical transport occurs though advection, eddy diffusion, sedimentation for both droplets and condensation nuclei. The cloud model is used to explore the sensitivity of Venus' cloud layer to environmental changes. Observations of the Venus' lower cloud from the Pioneer Venus, Venera, and Galileo spacecraft have suggested that the properties of the lower cloud may be time-variable, and at times may be entirely absent (Carlson et al. 1993, Grinspoon et al. 1993, Esposito et al. 1997). Our model explores the dependence of such behavior on environment factors such as variations in water or SO2 abundance. We have also calculated the optical properties of the model atmosphere using both the conventional optical constants for H2SO4 (Palmer and Williams, 1975), and the new data of Tisdale et al. (1998). This work has been supported by NASA's Exobiology Program. References Carlson, R.W., et al., 1993. Planetary and Space Science, 41, 477-486. Esposito, L.W., et al., 1997. In Venus II, eds. S.W. Bougher et al., pp. 415-458, University of Arizona Press, Tucson. Grinspoon, D.H., et al., 1993. Planetary and Space Science, 41 (July 1993), 515-542. James, E. P., et al., 1997. Icarus, 129, 147-171. Palmer, K.F., and D. Williams, 1975. Applied Optics, 14, 208-219. Tisdale, R.T., et al., 1998. Journal of Geophysical Research, 103, 25,353-25,370. Toon , O. B., et al., 1988. J. Atmos. Sci., 45, 2123-2143.

Thermodynamics and Dynamics of Bose condensation in a quasi-homogeneous gas

NASA Astrophysics Data System (ADS)

Navon, Nir; Schmidutz, Tobias; Gotlibovych, Igor; Gaunt, Alexander; Robert-de-Saint-Vincent, Martin; Smith, Robert; Hadzibabic, Zoran

2014-05-01

We present an experimental study of the thermodynamics and dynamics of Bose-Einstein condensation (BEC) in an optical-box trap. We first characterize the critical point for BEC, and observe saturation of the thermal component in a partially condensed cloud, in agreement with Einstein's textbook picture of a purely statistical phase transition. We also observed the quantum Joule-Thomson effect, namely isoenthalpic cooling of a non-interacting gas. We then investigate the dynamics of Bose condensation in the box potential following a rapid temperature quench through the phase transition, and focus on the time-evolution of the condensed fraction, the coherence length and the mean-field shift, that we probe via Bragg spectroscopy.

Strong impacts on aerosol indirect effects from historical oxidant changes

NASA Astrophysics Data System (ADS)

Hafsahl Karset, Inger Helene; Koren Berntsen, Terje; Storelvmo, Trude; Alterskjær, Kari; Grini, Alf; Olivié, Dirk; Kirkevåg, Alf; Seland, Øyvind; Iversen, Trond; Schulz, Michael

2018-06-01

Uncertainties in effective radiative forcings through aerosol-cloud interactions (ERFaci, also called aerosol indirect effects) contribute strongly to the uncertainty in the total preindustrial-to-present-day anthropogenic forcing. Some forcing estimates of the total aerosol indirect effect are so negative that they even offset the greenhouse gas forcing. This study highlights the role of oxidants in modeling of preindustrial-to-present-day aerosol indirect effects. We argue that the aerosol precursor gases should be exposed to oxidants of its era to get a more correct representation of secondary aerosol formation. Our model simulations show that the total aerosol indirect effect changes from -1.32 to -1.07 W m-2 when the precursor gases in the preindustrial simulation are exposed to preindustrial instead of present-day oxidants. This happens because of a brightening of the clouds in the preindustrial simulation, mainly due to large changes in the nitrate radical (NO3). The weaker oxidative power of the preindustrial atmosphere extends the lifetime of the precursor gases, enabling them to be transported higher up in the atmosphere and towards more remote areas where the susceptibility of the cloud albedo to aerosol changes is high. The oxidation changes also shift the importance of different chemical reactions and produce more condensate, thus increasing the size of the aerosols and making it easier for them to activate as cloud condensation nuclei.

Effects of turbulence on warm clouds and precipitation with various aerosol concentrations

NASA Astrophysics Data System (ADS)

Lee, Hyunho; Baik, Jong-Jin; Han, Ji-Young

2015-02-01

This study investigates the effects of turbulence-induced collision enhancement (TICE) on warm clouds and precipitation by changing the cloud condensation nuclei (CCN) number concentration using a two-dimensional dynamic model with bin microphysics. TICE is determined according to the Taylor microscale Reynolds number and the turbulent dissipation rate. The thermodynamic sounding used in this study is characterized by a warm and humid atmosphere with a capping inversion layer, which is suitable for simulating warm clouds. For all CCN concentrations, TICE slightly reduces the liquid water path during the early stage of cloud development and accelerates the onset of surface precipitation. However, changes in the rainwater path and in the amount of surface precipitation that are caused by TICE depend on the CCN concentrations. For high CCN concentrations, the mean cloud drop number concentration (CDNC) decreases and the mean effective radius increases due to TICE. These changes cause an increase in the amount of surface precipitation. However, for low CCN concentrations, changes in the mean CDNC and in the mean effective radius induced by TICE are small and the amount of surface precipitation decreases slightly due to TICE. A decrease in condensation due to the accelerated coalescence between droplets explains the surface precipitation decrease. In addition, an increase in the CCN concentration can lead to an increase in the amount of surface precipitation, and the relationship between the CCN concentration and the amount of surface precipitation is affected by TICE. It is shown that these results depend on the atmospheric relative humidity.

Sensitivities of simulated satellite views of clouds to subgrid-scale overlap and condensate heterogeneity

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hillman, Benjamin R.; Marchand, Roger T.; Ackerman, Thomas P.

Satellite simulators are often used to account for limitations in satellite retrievals of cloud properties in comparisons between models and satellite observations. The purpose of the simulator framework is to enable more robust evaluation of model cloud properties, so that di erences between models and observations can more con dently be attributed to model errors. However, these simulators are subject to uncertainties themselves. A fundamental uncertainty exists in connecting the spatial scales at which cloud properties are retrieved with those at which clouds are simulated in global models. In this study, we create a series of sensitivity tests using 4more » km global model output from the Multiscale Modeling Framework to evaluate the sensitivity of simulated satellite retrievals when applied to climate models whose grid spacing is many tens to hundreds of kilometers. In particular, we examine the impact of cloud and precipitation overlap and of condensate spatial variability. We find the simulated retrievals are sensitive to these assumptions. Specifically, using maximum-random overlap with homogeneous cloud and precipitation condensate, which is often used in global climate models, leads to large errors in MISR and ISCCP-simulated cloud cover and in CloudSat-simulated radar reflectivity. To correct for these errors, an improved treatment of unresolved clouds and precipitation is implemented for use with the simulator framework and is shown to substantially reduce the identified errors.« less

Evolution of the Far-Infrared Cloud at Titan's South Pole

NASA Technical Reports Server (NTRS)

Jennings, Donald E.; Achterberg, R. K.; Cottini, V.; Anderson, C. M.; Flasar, F. M.; Nixon, C. A.; Bjoraker, G. L.; Kunde, V. G.; Carlson, R. C.; Guandique, E.;

The case against climate regulation via oceanic phytoplankton sulphur emissions.

PubMed

Quinn, P K; Bates, T S

2011-11-30

More than twenty years ago, a biological regulation of climate was proposed whereby emissions of dimethyl sulphide from oceanic phytoplankton resulted in the formation of aerosol particles that acted as cloud condensation nuclei in the marine boundary layer. In this hypothesis--referred to as CLAW--the increase in cloud condensation nuclei led to an increase in cloud albedo with the resulting changes in temperature and radiation initiating a climate feedback altering dimethyl sulphide emissions from phytoplankton. Over the past two decades, observations in the marine boundary layer, laboratory studies and modelling efforts have been conducted seeking evidence for the CLAW hypothesis. The results indicate that a dimethyl sulphide biological control over cloud condensation nuclei probably does not exist and that sources of these nuclei to the marine boundary layer and the response of clouds to changes in aerosol are much more complex than was recognized twenty years ago. These results indicate that it is time to retire the CLAW hypothesis.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fan, Jiwen; Rosenfeld, Daniel; Zhang, Yuwei

Aerosol-cloud interactions remain the largest uncertainty in climate projections. Ultrafine aerosol particles smaller than 50 nanometers (UAP <50) can be abundant in the troposphere, but are conventionally considered too small to affect cloud formation. However, observational evidence and numerical simulations of deep convective clouds (DCCs) over the Amazon show that DCCs forming in a low aerosol environment can develop very large vapor supersaturation because fast droplet coalescence reduces integrated droplet surface area and subsequent condensation. UAP <50 from pollution plumes that are ingested into such clouds can be activated to form additional cloud droplets on which excess supersaturation condenses andmore » forms additional cloud water and latent heating, thus intensifying convective strength. This mechanism suggests a strong anthropogenic invigoration of DCCs in previously pristine regions of the world.« less

Aerosol partitioning between the interstitial and the condensed phase in mixed-phase clouds

NASA Astrophysics Data System (ADS)

Verheggen, Bart; Cozic, Julie; Weingartner, Ernest; Bower, Keith; Mertes, Stephan; Connolly, Paul; Gallagher, Martin; Flynn, Michael; Choularton, Tom; Baltensperger, Urs

2007-12-01

The partitioning of aerosol particles between the cloud and the interstitial phase (i.e., unactivated aerosol) has been investigated during several Cloud and Aerosol Characterization Experiments (CLACE-3, CLACE-3? and CLACE-4) conducted in winter and summer 2004 and winter 2005 at the high alpine research station Jungfraujoch (3580 m altitude, Switzerland). Ambient air was sampled using different inlets in order to determine the activated fraction of aerosol particles, FN, defined as the fraction of the total aerosol number concentration (with particle diameter dp > 100 nm) that has been incorporated into cloud particles. The liquid and ice water content of mixed-phase clouds were characterized by analyzing multiple cloud probes. The dependence of the activated fraction on several environmental factors is discussed on the basis of more than 900 h of in-cloud observations and parameterizations for key variables are given. FN is found to increase with increasing liquid water content and to decrease with increasing particle number concentration in liquid clouds. FN also decreases with increasing cloud ice mass fraction and with decreasing temperature from 0 to -25°C. The Wegener-Bergeron-Findeisen process probably contributed to this trend, since the presence of ice crystals causes liquid droplets to evaporate, thus releasing the formerly activated particles back into the interstitial phase. Ice nucleation could also have prevented additional cloud condensation nuclei from activating. The observed activation behavior has significant implications for our understanding of the indirect effect of aerosols on climate.

An observational search for CO2 ice clouds on Mars

NASA Technical Reports Server (NTRS)

Bell, James F., III; Calvin, Wendy M.; Pollack, James B.; Crisp, David

1993-01-01

CO2 ice clouds were first directly identified on Mars by the Mariner 6 and 7 infrared spectrometer limb scans. These observations provided support for early theoretical modeling efforts of CO2 condensation. Mariner 9 IRIS temperature profiles of north polar hood clouds were interpreted as indicating that these clouds were composed of H2O ice at lower latitudes and CO2 ice at higher latitudes. The role of CO2 condensation on Mars has recently received increased attention because (1) Kasting's model results indicated that CO2 cloud condensation limits the magnitude of the proposed early Mars CO2/H2O greenhouse, and (2) Pollack el al.'s GCM results indicated that the formation of CO2 ice clouds is favorable at all polar latitudes during the fall and winter seasons. These latter authors have shown that CO2 clouds play an important role in the polar energy balance, as the amount of CO2 contained in the polar caps is constrained by a balance between latent heat release, heat advected from lower latitudes, and thermal emission to space. The polar hood clouds reduce the amount of CO2 condensation on the polar caps because they reduce the net emission to space. There have been many extensive laboratory spectroscopic studies of H2O and CO2 ices and frosts. In this study, we use results from these and other sources to search for the occurrence of diagnostic CO2 (and H2O) ice and/or frost absorption features in ground based near-infrared imaging spectroscopic data of Mars. Our primary goals are (1) to try to confirm the previous direct observations of CO2 clouds on Mars; (2) to determine the spatial extent, temporal variability, and composition (H2O/CO2 ratio) of any clouds detected; and (3) through radiative transfer modeling, to try to determine the mean particle size and optical depth of polar hood clouds, thus, assessing their role in the polar heat budget.

Sedimentation Efficiency of Condensation Clouds in Substellar Atmospheres

NASA Astrophysics Data System (ADS)

Gao, Peter; Marley, Mark S.; Ackerman, Andrew S.

2018-03-01

Condensation clouds in substellar atmospheres have been widely inferred from spectra and photometric variability. Up until now, their horizontally averaged vertical distribution and mean particle size have been largely characterized using models, one of which is the eddy diffusion–sedimentation model from Ackerman and Marley that relies on a sedimentation efficiency parameter, f sed, to determine the vertical extent of clouds in the atmosphere. However, the physical processes controlling the vertical structure of clouds in substellar atmospheres are not well understood. In this work, we derive trends in f sed across a large range of eddy diffusivities (K zz ), gravities, material properties, and cloud formation pathways by fitting cloud distributions calculated by a more detailed cloud microphysics model. We find that f sed is dependent on K zz , but not gravity, when K zz is held constant. f sed is most sensitive to the nucleation rate of cloud particles, as determined by material properties like surface energy and molecular weight. High surface energy materials form fewer, larger cloud particles, leading to large f sed (>1), and vice versa for materials with low surface energy. For cloud formation via heterogeneous nucleation, f sed is sensitive to the condensation nuclei flux and radius, connecting cloud formation in substellar atmospheres to the objects’ formation environments and other atmospheric aerosols. These insights could lead to improved cloud models that help us better understand substellar atmospheres. For example, we demonstrate that f sed could increase with increasing cloud base depth in an atmosphere, shedding light on the nature of the brown dwarf L/T transition.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fan, Jiwen; Rosenfeld, Daniel; Zhang, Yuwei

Aerosol-cloud interaction remains the largest uncertainty in climate projections. Ultrafine aerosol particles (UAP; size <50nm) are considered too small to serve as cloud condensation nuclei conventionally. However, this study provides observational evidence to accompany insights from numerical simulations to support that deep convective clouds (DCCs) over Amazon have strong capability of nucleating UAP from an urban source and forming greater numbers of droplets, because fast drop coalescence in these DCCs reduces drop surface area available for condensation, leading to high vapor supersaturation. The additional droplets subsequently decrease supersaturation and release more condensational latent heating, a dominant contributor to convection intensification,more » whereas enhanced latent heat from ice-related processes plays a secondary role. Therefore, the addition of anthropogenic UAP may play a much greater role in modulating clouds than previously believed over the Amazon region and possibly in other relatively pristine regions such as maritime and forest locations.« less

Cloud Atlas: Rotational Modulations in the L/T Transition Brown Dwarf Companion HN Peg B

NASA Technical Reports Server (NTRS)

Zhou, Yifan; Apai, Daniel; Metchev, Stanimir; Lew, Ben W. P.; Schneider, Glenn; Marley, Mark S.; Karalidi, Theodora; Manjavacas, Elena; Bedin, Luigi R.; Cowan, Nicolas B.;

Cloud Atlas: Rotational Modulations in the L/T Transition Brown Dwarf Companion HN Peg B

NASA Astrophysics Data System (ADS)

Zhou, Yifan; Apai, Dániel; Metchev, Stanimir; Lew, Ben W. P.; Schneider, Glenn; Marley, Mark S.; Karalidi, Theodora; Manjavacas, Elena; Bedin, Luigi R.; Cowan, Nicolas B.; Miles-Páez, Paulo A.; Lowrance, Patrick J.; Radigan, Jacqueline; Burgasser, Adam J.

2018-03-01

Time-resolved observations of brown dwarfs’ rotational modulations provide powerful insights into the properties of condensate clouds in ultra-cool atmospheres. Multi-wavelength light curves reveal cloud vertical structures, condensate particle sizes, and cloud morphology, which directly constrain condensate cloud and atmospheric circulation models. We report results from Hubble Space Telescope/Wide Field Camera 3 near-infrared G141 taken in six consecutive orbits observations of HN Peg B, an L/T transition brown dwarf companion to a G0V type star. The best-fit sine wave to the 1.1–1.7 μm broadband light curve has an amplitude of 1.206% ± 0.025% and period of 15.4 ± 0.5 hr. The modulation amplitude has no detectable wavelength dependence except in the 1.4 μm water absorption band, indicating that the characteristic condensate particle sizes are large (>1 μm). We detect significantly (4.4σ) lower modulation amplitude in the 1.4 μm water absorption band and find that HN Peg B’s spectral modulation resembles those of early T type brown dwarfs. We also describe a new empirical interpolation method to remove spectral contamination from the bright host star. This method may be applied in other high-contrast time-resolved observations with WFC3.

On the Effect of Dust Particles on Global Cloud Condensation Nuclei and Cloud Droplet Number

NASA Technical Reports Server (NTRS)

Karydis, V. A.; Kumar, P.; Barahona, D.; Sokolik, I. N.; Nenes, A.

2011-01-01

Aerosol-cloud interaction studies to date consider aerosol with a substantial fraction of soluble material as the sole source of cloud condensation nuclei (CCN). Emerging evidence suggests that mineral dust can act as good CCN through water adsorption onto the surface of particles. This study provides a first assessment of the contribution of insoluble dust to global CCN and cloud droplet number concentration (CDNC). Simulations are carried out with the NASA Global Modeling Initiative chemical transport model with an online aerosol simulation, considering emissions from fossil fuel, biomass burning, marine, and dust sources. CDNC is calculated online and explicitly considers the competition of soluble and insoluble CCN for water vapor. The predicted annual average contribution of insoluble mineral dust to CCN and CDNC in cloud-forming areas is up to 40 and 23.8%, respectively. Sensitivity tests suggest that uncertainties in dust size distribution and water adsorption parameters modulate the contribution of mineral dust to CDNC by 23 and 56%, respectively. Coating of dust by hygroscopic salts during the atmospheric aging causes a twofold enhancement of the dust contribution to CCN; the aged dust, however, can substantially deplete in-cloud supersaturation during the initial stages of cloud formation and can eventually reduce CDNC. Considering the hydrophilicity from adsorption and hygroscopicity from solute is required to comprehensively capture the dust-warm cloud interactions. The framework presented here addresses this need and can be easily integrated in atmospheric models.

Biogenic Potassium Salt Particles as Seeds for Secondary Organic Aerosol in the Amazon

NASA Astrophysics Data System (ADS)

Pöhlker, Christopher; Wiedemann, Kenia T.; Sinha, Bärbel; Shiraiwa, Manabu; Gunthe, Sachin S.; Smith, Mackenzie; Su, Hang; Artaxo, Paulo; Chen, Qi; Cheng, Yafang; Elbert, Wolfgang; Gilles, Mary K.; Kilcoyne, Arthur L. D.; Moffet, Ryan C.; Weigand, Markus; Martin, Scot T.; Pöschl, Ulrich; Andreae, Meinrat O.

2012-08-01

The fine particles serving as cloud condensation nuclei in pristine Amazonian rainforest air consist mostly of secondary organic aerosol. Their origin is enigmatic, however, because new particle formation in the atmosphere is not observed. Here, we show that the growth of organic aerosol particles can be initiated by potassium-salt-rich particles emitted by biota in the rainforest. These particles act as seeds for the condensation of low- or semi-volatile organic compounds from the atmospheric gas phase or multiphase oxidation of isoprene and terpenes. Our findings suggest that the primary emission of biogenic salt particles directly influences the number concentration of cloud condensation nuclei and affects the microphysics of cloud formation and precipitation over the rainforest.

How do changes in warm-phase microphysics affect deep convective clouds?

NASA Astrophysics Data System (ADS)

Chen, Qian; Koren, Ilan; Altaratz, Orit; Heiblum, Reuven H.; Dagan, Guy; Pinto, Lital

2017-08-01

Understanding aerosol effects on deep convective clouds and the derived effects on the radiation budget and rain patterns can largely contribute to estimations of climate uncertainties. The challenge is difficult in part because key microphysical processes in the mixed and cold phases are still not well understood. For deep convective clouds with a warm base, understanding aerosol effects on the warm processes is extremely important as they set the initial and boundary conditions for the cold processes. Therefore, the focus of this study is the warm phase, which can be better resolved. The main question is: How do aerosol-derived changes in the warm phase affect the properties of deep convective cloud systems? To explore this question, we used a weather research and forecasting (WRF) model with spectral bin microphysics to simulate a deep convective cloud system over the Marshall Islands during the Kwajalein Experiment (KWAJEX). The model results were validated against observations, showing similarities in the vertical profile of radar reflectivity and the surface rain rate. Simulations with larger aerosol loading resulted in a larger total cloud mass, a larger cloud fraction in the upper levels, and a larger frequency of strong updrafts and rain rates. Enlarged mass both below and above the zero temperature level (ZTL) contributed to the increase in cloud total mass (water and ice) in the polluted runs. Increased condensation efficiency of cloud droplets governed the gain in mass below the ZTL, while both enhanced condensational and depositional growth led to increased mass above it. The enhanced mass loading above the ZTL acted to reduce the cloud buoyancy, while the thermal buoyancy (driven by the enhanced latent heat release) increased in the polluted runs. The overall effect showed an increased upward transport (across the ZTL) of liquid water driven by both larger updrafts and larger droplet mobility. These aerosol effects were reflected in the larger ratio between the masses located above and below the ZTL in the polluted runs. When comparing the net mass flux crossing the ZTL in the clean and polluted runs, the difference was small. However, when comparing the upward and downward fluxes separately, the increase in aerosol concentration was seen to dramatically increase the fluxes in both directions, indicating the aerosol amplification effect of the convection and the affected cloud system properties, such as cloud fraction and rain rate.

Effects of cloud condensation nuclei and ice nucleating particles on precipitation processes and supercooled liquid in mixed-phase orographic clouds

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fan, Jiwen; Leung, L. Ruby; Rosenfeld, Daniel

How orographic mixed-phase clouds respond to the change in cloud condensation nuclei (CCN) and ice nucleating particles (INPs) are highly uncertain. The main snow production mechanism in warm and cold mixed-phase orographic clouds (referred to as WMOCs and CMOCs, respectively, distinguished here as those having cloud tops warmer and colder than -20°C) could be very different. We quantify the CCN and INP impacts on supercooled water content, cloud phases, and precipitation for a WMOC case and a CMOC case, with sensitivity tests using the same CCN and INP concentrations between the WMOC and CMOC cases. It was found that depositionmore » plays a more important role than riming for forming snow in the CMOC case, while the role of riming is dominant in the WMOC case. As expected, adding CCN suppresses precipitation, especially in WMOCs and low INPs. However, this reverses strongly for CCN of 1000 cm -3 and larger. We found a new mechanism through which CCN can invigorate mixed-phase clouds over the Sierra Nevada and drastically intensify snow precipitation when CCN concentrations are high (1000 cm -3 or higher). In this situation, more widespread shallow clouds with a greater amount of cloud water form in the Central Valley and foothills west of the mountain range. The increased latent heat release associated with the formation of these clouds strengthens the local transport of moisture to the windward slope, invigorating mixed-phase clouds over the mountains, and thereby producing higher amounts of snow precipitation. Under all CCN conditions, increasing the INPs leads to decreased riming and mixed-phase fraction in the CMOC as a result of liquid-limited conditions, but has the opposite effects in the WMOC as a result of ice-limited conditions. However, precipitation in both cases is increased by increasing INPs due to an increase in deposition for the CMOC but enhanced riming and deposition in the WMOC. Increasing the INPs dramatically reduces supercooled water content and increases the cloud glaciation temperature, while increasing CCN has the opposite effect with much smaller significance.« less

Effects of cloud condensation nuclei and ice nucleating particles on precipitation processes and supercooled liquid in mixed-phase orographic clouds

DOE PAGES

Fan, Jiwen; Leung, L. Ruby; Rosenfeld, Daniel; ...

2017-01-23

How orographic mixed-phase clouds respond to the change in cloud condensation nuclei (CCN) and ice nucleating particles (INPs) are highly uncertain. The main snow production mechanism in warm and cold mixed-phase orographic clouds (referred to as WMOCs and CMOCs, respectively, distinguished here as those having cloud tops warmer and colder than -20°C) could be very different. We quantify the CCN and INP impacts on supercooled water content, cloud phases, and precipitation for a WMOC case and a CMOC case, with sensitivity tests using the same CCN and INP concentrations between the WMOC and CMOC cases. It was found that depositionmore » plays a more important role than riming for forming snow in the CMOC case, while the role of riming is dominant in the WMOC case. As expected, adding CCN suppresses precipitation, especially in WMOCs and low INPs. However, this reverses strongly for CCN of 1000 cm -3 and larger. We found a new mechanism through which CCN can invigorate mixed-phase clouds over the Sierra Nevada and drastically intensify snow precipitation when CCN concentrations are high (1000 cm -3 or higher). In this situation, more widespread shallow clouds with a greater amount of cloud water form in the Central Valley and foothills west of the mountain range. The increased latent heat release associated with the formation of these clouds strengthens the local transport of moisture to the windward slope, invigorating mixed-phase clouds over the mountains, and thereby producing higher amounts of snow precipitation. Under all CCN conditions, increasing the INPs leads to decreased riming and mixed-phase fraction in the CMOC as a result of liquid-limited conditions, but has the opposite effects in the WMOC as a result of ice-limited conditions. However, precipitation in both cases is increased by increasing INPs due to an increase in deposition for the CMOC but enhanced riming and deposition in the WMOC. Increasing the INPs dramatically reduces supercooled water content and increases the cloud glaciation temperature, while increasing CCN has the opposite effect with much smaller significance.« less

Substantial convection and precipitation enhancements by ultrafine aerosol particles

DOE PAGES

Fan, Jiwen; Rosenfeld, Daniel; Zhang, Yuwei; ...

2018-01-26

Aerosol-cloud interactions remain the largest uncertainty in climate projections. Ultrafine aerosol particles smaller than 50 nanometers (UAP <50) can be abundant in the troposphere, but are conventionally considered too small to affect cloud formation. However, observational evidence and numerical simulations of deep convective clouds (DCCs) over the Amazon show that DCCs forming in a low aerosol environment can develop very large vapor supersaturation because fast droplet coalescence reduces integrated droplet surface area and subsequent condensation. UAP <50 from pollution plumes that are ingested into such clouds can be activated to form additional cloud droplets on which excess supersaturation condenses andmore » forms additional cloud water and latent heating, thus intensifying convective strength. This mechanism suggests a strong anthropogenic invigoration of DCCs in previously pristine regions of the world.« less

Process-model simulations of cloud albedo enhancement by aerosols in the Arctic.

PubMed

Kravitz, Ben; Wang, Hailong; Rasch, Philip J; Morrison, Hugh; Solomon, Amy B

2014-12-28

A cloud-resolving model is used to simulate the effectiveness of Arctic marine cloud brightening via injection of cloud condensation nuclei (CCN), either through geoengineering or other increased sources of Arctic aerosols. An updated cloud microphysical scheme is employed, with prognostic CCN and cloud particle numbers in both liquid and mixed-phase marine low clouds. Injection of CCN into the marine boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. Albedo increases are stronger for pure liquid clouds than mixed-phase clouds. Liquid precipitation can be suppressed by CCN injection, whereas ice precipitation (snow) is affected less; thus, the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. CCN injection into a clean regime results in a greater albedo increase than injection into a polluted regime, consistent with current knowledge about aerosol-cloud interactions. Unlike previous studies investigating warm clouds, dynamical changes in circulation owing to precipitation changes are small. According to these results, which are dependent upon the representation of ice nucleation processes in the employed microphysical scheme, Arctic geoengineering is unlikely to be effective as the sole means of altering the global radiation budget but could have substantial local radiative effects. © 2014 The Author(s) Published by the Royal Society. All rights reserved.

Process-model simulations of cloud albedo enhancement by aerosols in the Arctic

PubMed Central

Kravitz, Ben; Wang, Hailong; Rasch, Philip J.; Morrison, Hugh; Solomon, Amy B.

2014-01-01

A cloud-resolving model is used to simulate the effectiveness of Arctic marine cloud brightening via injection of cloud condensation nuclei (CCN), either through geoengineering or other increased sources of Arctic aerosols. An updated cloud microphysical scheme is employed, with prognostic CCN and cloud particle numbers in both liquid and mixed-phase marine low clouds. Injection of CCN into the marine boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. Albedo increases are stronger for pure liquid clouds than mixed-phase clouds. Liquid precipitation can be suppressed by CCN injection, whereas ice precipitation (snow) is affected less; thus, the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. CCN injection into a clean regime results in a greater albedo increase than injection into a polluted regime, consistent with current knowledge about aerosol–cloud interactions. Unlike previous studies investigating warm clouds, dynamical changes in circulation owing to precipitation changes are small. According to these results, which are dependent upon the representation of ice nucleation processes in the employed microphysical scheme, Arctic geoengineering is unlikely to be effective as the sole means of altering the global radiation budget but could have substantial local radiative effects. PMID:25404677

Dimethylsulfide oxidation over the tropical South Atlantic: OH and other oxidants

NASA Technical Reports Server (NTRS)

Hemming, Brooke L.; Vastano, John A.; Chatfield, Robert B.; Andreae, Meinrat O.; Hildemann, Lynn M.

1994-01-01

The general course of events in the formation of a marine cloud begins with the emission of species which can eventually serve as nuclei around which water can condense to form a cloud droplet. In remote marine regions, cloud condensation nuclei (CCN) are primarily composed of sulfate, in either its acid or ammonium salt form. Most sulfate in these regions is the product of atmospheric oxidation of dimethyl sulfide (DMS), a reduced sulfur gas that is released by phytoplankton at the ocean surface. Therefore, in order to effectively quantify the links in the cloud-formation cycle, one must begin with a well-defined description of the atmospheric chemistry of DMS. The intent of this project has been to initiate development of a comprehensive model of the chemistry and dynamics responsible for the formation of clouds in the remote marine boundary layer. The primary tool in this work has been the Global/Regional Atmospheric Chemistry Event Simulator (GRACES), a global atmospheric chemistry model, which is under development within the Atmospheric Chemistry and Dynamics Branch of NASA-Ames Research Center. In this effort, GRACES was used to explore the first chemical link between DMS and sulfate by modeling the diurnal variation of DMS.

Combustion Organic Aerosol as Cloud Condensation Nuclei in Ship Tracks.

NASA Astrophysics Data System (ADS)

Russell, Lynn M.; Noone, Kevin J.; Ferek, Ronald J.; Pockalny, Robert A.; Flagan, Richard C.; Seinfeld, John H.

2000-08-01

Polycyclic aromatic hydrocarbons (PAHs) have been sampled in marine stratiform clouds to identify the contribution of anthropogenic combustion emissions in activation of aerosol to cloud droplets. The Monterey Area Ship Track experiment provided an opportunity to acquire data on the role of organic compounds in ambient clouds and in ship tracks identified in satellite images. Identification of PAHs in cloud droplet residual samples indicates that several PAHs are present in cloud condensation nuclei in anthropogenically influenced air and do result in activated droplets in cloud. These results establish the presence of combustion products, such as PAHs, in submicrometer aerosols in anthropogenically influenced marine air, with enhanced concentrations in air polluted by ship effluent. The presence of PAHs in droplet residuals in anthropogenically influenced air masses indicates that some fraction of those combustion products is present in the cloud condensation nuclei that activate in cloud. Although a sufficient mass of droplet residuals was not collected to establish a similar role for organics from measurements in satellite-identified ship tracks, the available evidence from the fraction of organics present in the interstitial aerosol is consistent with part of the organic fraction partitioning to the droplet population. In addition, the probability that a compound will be found in cloud droplets rather than in the unactivated aerosol and the compound's water solubility are compared. The PAHs studied are only weakly soluble in water, but most of the sparse data collected support more soluble compounds having a higher probability of activation.

Entrainment, Drizzle, and the Indirect Effect in Stratiform Clouds

NASA Technical Reports Server (NTRS)

Ackerman, Andrew

2005-01-01

Activation of some fraction of increased concentrations of sub-micron soluble aerosol particles lead to enhanced cloud droplet concentrations and hence smaller droplets, increasing their total cross sectional area and thus reflecting solar radiation more efficiently (the Twomey, or first indirect, effect). However, because of competition during condensational growth, droplet distributions tend to broaden as numbers increase, reducing the sensitivity of cloud albedo to droplet concentration on the order of 10%. Also, smaller droplets less effectively produce drizzle through collisions and coalescence, and it is widely expected (and found in large-scale models) that decreased precipitation leads to clouds with more cloud water on average (the so-called cloud lifetime, or second indirect, effect). Much of the uncertainty regarding the overall indirect aerosol effect stems from inadequate understanding of such changes in cloud water. Detailed simulations based on FIRE-I, ASTEX, and DYCOMS-II conditions show that suppression of precipitation from increased droplet concentrations leads to increased cloud water only when sufficient precipitation reaches the surface, a condition favored when the overlying air is-humid or droplet concentrations are very low. Otherwise, aerosol induced suppression of precipitation enhances entrainment of overlying dry air, thereby reducing cloud water and diminishing the indirect climate forcing.

Aerosol Production and Growth in the Upper Troposphere over the Amazon Forest Observed during ACRIDICON-CHUVA

NASA Astrophysics Data System (ADS)

Andreae, M. O.; Afchine, A.; Albrecht, R. I.; Artaxo, P.; Borrmann, S.; Cecchini, M. A.; Costa, A.; Fütterer, D.; Järvinen, E.; Klimach, T.; Konemann, T.; Kraemer, M.; Machado, L.; Mertes, S.; Pöhlker, C.; Pöhlker, M. L.; Poeschl, U.; Sauer, D. N.; Schnaiter, M.; Schneider, J.; Schulz, C.; Spanu, A.; Walser, A.; Wang, J.; Weinzierl, B.; Wendisch, M.

2016-12-01

Observations during ACRIDICON-CHUVA showed high aerosol concentrations in the upper troposphere (UT) over the Amazon Basin, with aerosol number concentrations after normalization to STP often exceeding those in the boundary layer (BL) by one or two orders of magnitude. The measurements were made during the German-Brazilian cooperative aircraft campaign ACRIDICON-CHUVA (Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems) on the German research aircraft HALO. The campaign took place over the Amazon Basin in September/October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with trace gases, aerosol particles, and atmospheric radiation. Aerosol enhancements were consistently observed on all flights, using several aerosol metrics, including condensation nuclei (CN), cloud condensation nuclei (CCN), and chemical species mass concentrations. These UT aerosols were different in their composition and size distribution from the aerosol in the BL, making convective transport of particles unlikely as a source. The regions in the immediate outflow of deep convective clouds were depleted in aerosol particles, whereas dramatically enhanced small (<90 nm diameter) aerosol number concentrations were found in UT regions that had experienced outflow from deep convection in the preceding 24-48 hours. We also found elevated concentrations of larger (>90 nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN. Our findings suggest that aerosol production takes place in the UT from volatile material brought up by deep convection, which is converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol may be a source of particles to the BL, where they increase in size by the condensation of biogenic volatile organic carbon (BVOC) oxidation products. This may be an important source of aerosol particles in the Amazonian BL, where aerosol nucleation and new particle formation has not been observed. We propose that this may have been the dominant process supplying secondary aerosols in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles.

Dust in brown dwarfs. III. Formation and structure of quasi-static cloud layers

NASA Astrophysics Data System (ADS)

Woitke, P.; Helling, Ch.

2004-01-01

In this paper, first solutions of the dust moment equations developed in (Woitke & Helling \\cite{wh2003a}) for the description of dust formation and precipitation in brown dwarf and giant gas planet atmospheres are presented. We consider the special case of a static brown dwarf atmosphere, where dust particles continuously nucleate from the gas phase, grow by the accretion of molecules, settle gravitationally and re-evaporate thermally. Mixing by convective overshoot is assumed to replenish the atmosphere with condensable elements, which is necessary to counterbalance the loss of condensable elements by dust formation and gravitational settling (no dust without mixing). Applying a kinetic description of the relevant microphysical and chemical processes for TiO2-grains, the model makes predictions about the large-scale stratification of dust in the atmosphere, the depletion of molecules from the gas phase, the supersaturation of the gas in the atmosphere as well as the mean size and the mass fraction of dust grains as function of depth. Our results suggest that the presence of relevant amounts of dust is restricted to a layer, where the upper boundary (cloud deck) is related to the requirement of a minimum mixing activity (mixing time-scale τmix ≈ 10 6 s) and the lower boundary (cloud base) is determined by the thermodynamical stability of the grains. The nucleation occurs around the cloud deck where the gas is cool, strongly depleted, but nevertheless highly supersaturated (S ≫ 1). These particles settle gravitationally and populate the warmer layers below, where the in situ formation (nucleation) is ineffective or even not possible. During their descent, the particles grow and reach mean radii of ≈30 \\mum ... 400 \\mum at the cloud base, but the majority of the particles in the cloud layer remains much smaller. Finally, the dust grains sink into layers which are sufficiently hot to cause their thermal evaporation. Hence, an effective transport mechanism for condensable elements exists in brown dwarfs, which depletes the gas above and enriches the gas below the cloud base of a considered solid/liquid material. The dust-to-gas mass fraction in the cloud layer results to be approximately given by the mass fraction of condensable elements in the gas being mixed up. Only for artificially reduced mixing we find a self-regulation mechanism that approximately installs phase equilibrium (S ≈ 1) in a limited region around the cloud base.

Lagrangian condensation microphysics with Twomey CCN activation

NASA Astrophysics Data System (ADS)

Grabowski, Wojciech W.; Dziekan, Piotr; Pawlowska, Hanna

2018-01-01

We report the development of a novel Lagrangian microphysics methodology for simulations of warm ice-free clouds. The approach applies the traditional Eulerian method for the momentum and continuous thermodynamic fields such as the temperature and water vapor mixing ratio, and uses Lagrangian super-droplets to represent condensed phase such as cloud droplets and drizzle or rain drops. In other applications of the Lagrangian warm-rain microphysics, the super-droplets outside clouds represent unactivated cloud condensation nuclei (CCN) that become activated upon entering a cloud and can further grow through diffusional and collisional processes. The original methodology allows for the detailed study of not only effects of CCN on cloud microphysics and dynamics, but also CCN processing by a cloud. However, when cloud processing is not of interest, a simpler and computationally more efficient approach can be used with super-droplets forming only when CCN is activated and no super-droplet existing outside a cloud. This is possible by applying the Twomey activation scheme where the local supersaturation dictates the concentration of cloud droplets that need to be present inside a cloudy volume, as typically used in Eulerian bin microphysics schemes. Since a cloud volume is a small fraction of the computational domain volume, the Twomey super-droplets provide significant computational advantage when compared to the original super-droplet methodology. Additional advantage comes from significantly longer time steps that can be used when modeling of CCN deliquescence is avoided. Moreover, other formulation of the droplet activation can be applied in case of low vertical resolution of the host model, for instance, linking the concentration of activated cloud droplets to the local updraft speed. This paper discusses the development and testing of the Twomey super-droplet methodology, focusing on the activation and diffusional growth. Details of the activation implementation, transport of super-droplets in the physical space, and the coupling between super-droplets and the Eulerian temperature and water vapor field are discussed in detail. Some of these are relevant to the original super-droplet methodology as well and to the ice phase modeling using the Lagrangian approach. As a computational example, the scheme is applied to an idealized moist thermal rising in a stratified environment, with the original super-droplet methodology providing a benchmark to which the new scheme is compared.

New approaches to quantifying aerosol influence on the cloud radiative effect

DOE PAGES

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; ...

2016-02-01

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol–cloud interactions at ever-increasing levels of detail, but these models lack the resolution tomore » represent clouds and aerosol–cloud interactions adequately. There is a dearth of observational constraints on aerosol–cloud interactions. In this paper, we develop a conceptual approach to systematically constrain the aerosol–cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. Finally, we heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol–cloud radiation system.« less

New approaches to quantifying aerosol influence on the cloud radiative effect

PubMed Central

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; Johnson, Jill S.; Carslaw, Kenneth S.; Schmidt, K. Sebastian

2016-01-01

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol−cloud interactions at ever-increasing levels of detail, but these models lack the resolution to represent clouds and aerosol−cloud interactions adequately. There is a dearth of observational constraints on aerosol−cloud interactions. We develop a conceptual approach to systematically constrain the aerosol−cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. We heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol−cloud radiation system. PMID:26831092

New approaches to quantifying aerosol influence on the cloud radiative effect.

PubMed

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; Johnson, Jill S; Carslaw, Kenneth S; Schmidt, K Sebastian

2016-05-24

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol-cloud interactions at ever-increasing levels of detail, but these models lack the resolution to represent clouds and aerosol-cloud interactions adequately. There is a dearth of observational constraints on aerosol-cloud interactions. We develop a conceptual approach to systematically constrain the aerosol-cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. We heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol-cloud radiation system.

Venus: Halide cloud condensation and volatile element inventories

NASA Technical Reports Server (NTRS)

Lewis, J. S.; Fegley, B., Jr.

1982-01-01

Several Venus cloud condensates, including A12C16 as well as halides, oxides and sulfides of arsenic and antimony, are assessed for their thermodynamic and geochemical plausibility. Aluminum chloride can confidently be ruled out, and condensation of arsenic sulfides on the surface will cause arsenic compounds to be too rare to produce the observed clouds. Antimony may conceivably be sufficiently volatile, but the expected molecular form is gaseous SbS, not the chloride. Arsenic and antimony compounds in the atmosphere will be regulated at very low levels by sulfide precipitation, irrespective of the planetary inventory of As and Sb. Thus the arguments for a volatile-deficient origin for Venus based on the depletion of water and mercury (relative to Earth) cannot be tested by a search for atmospheric arsenic or antimony.

Urbanization Causes Increased Cloud Base Height and Decreased Fog in Coastal Southern California

NASA Technical Reports Server (NTRS)

Williams, A. Park; Schwartz, Rachel E.; Iacobellis, Sam; Seager, Richard; Cook, Benjamin I.; Still, Christopher J.; Husak, Gregory; Michaelsen, Joel

2015-01-01

Subtropical marine stratus clouds regulate coastal and global climate, but future trends in these clouds are uncertain. In coastal Southern California (CSCA), interannual variations in summer stratus cloud occurrence are spatially coherent across 24 airfields and dictated by positive relationships with stability above the marine boundary layer (MBL) and MBL height. Trends, however, have been spatially variable since records began in the mid-1900s due to differences in nighttime warming. Among CSCA airfields, differences in nighttime warming, but not daytime warming, are strongly and positively related to fraction of nearby urban cover, consistent with an urban heat island effect. Nighttime warming raises the near-surface dew point depression, which lifts the altitude of condensation and cloud base height, thereby reducing fog frequency. Continued urban warming, rising cloud base heights, and associated effects on energy and water balance would profoundly impact ecological and human systems in highly populated and ecologically diverse CSCA.

A microphysical parameterization of aqSOA and sulfate formation in clouds

NASA Astrophysics Data System (ADS)

McVay, Renee; Ervens, Barbara

2017-07-01

Sulfate and secondary organic aerosol (cloud aqSOA) can be chemically formed in cloud water. Model implementation of these processes represents a computational burden due to the large number of microphysical and chemical parameters. Chemical mechanisms have been condensed by reducing the number of chemical parameters. Here an alternative is presented to reduce the number of microphysical parameters (number of cloud droplet size classes). In-cloud mass formation is surface and volume dependent due to surface-limited oxidant uptake and/or size-dependent pH. Box and parcel model simulations show that using the effective cloud droplet diameter (proportional to total volume-to-surface ratio) reproduces sulfate and aqSOA formation rates within ≤30% as compared to full droplet distributions; other single diameters lead to much greater deviations. This single-class approach reduces computing time significantly and can be included in models when total liquid water content and effective diameter are available.

Deployment of ARM Aerial Facility Scanning Mobility Particle Sizer Field Campaign Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, Jian

2016-09-01

Atmospheric aerosols influence global climate by scattering and absorbing sunlight (direct effects) and by changing the microphysical structure, lifetime, and coverage of clouds (indirect effects). While it is widely accepted that aerosol indirect effects cool the Earth-atmosphere system by increasing cloud reflectivity and coverage, the magnitudes of the indirect effects are poorly quantified. One key aerosol property for understanding aerosol indirect effects is the ability of aerosol particles to form cloud droplets at atmospheric relevant supersaturations—i.e., cloud condensation Nuclei (CCN) activity. For particles consisting of typical atmospheric inorganic compounds, their CCN activity is well understood and can be effectively predictedmore » using Köhler theory based on physicochemical properties of the solute, such as its mass, molar volume, and activity coefficient. However, atmospheric aerosols often consist of hundreds of organic species, which can contribute ~20-90% to the total fine aerosol mass. Depending on their properties, organic species can significantly influence the ability of aerosol particles to act as CCN and form cloud droplets. This project focuses on the CCN activity of secondary organic aerosol (SOA) compounds formed from key biogenic volatile organic compounds (VOCs) under representative conditions, and the relationship between the hygroscopicity and composition of organic aerosols. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility Aerial Facility (AAF) scanning mobility particles sizer (SMPS) was deployed during a ~ 2-week intensive measurement campaign, taking place February 10-February 23, 2016 at the Pacific Northwest National Laboratory (PNNL) Environmental Simulation Chamber. The SMPS was operated with a CCN counter (CCNc). Aerosol particles were first classified by the differential mobility analyzer inside the SMPS; the classified aerosol will then be simultaneously characterized by a condensation particle counter (CPC) (part of the SMPS) and the CCNc.« less

Aerosol Enhancements in the Upper Troposphere Over The Amazon Forest: Do Amazonian Clouds Produce Aerosols?

NASA Astrophysics Data System (ADS)

Andreae, M. O.; Afchine, A.; Albrecht, R. I.; Artaxo, P.; Borrmann, S.; Cecchini, M. A.; Costa, A.; Dollner, M.; Fütterer, D.; Järvinen, E.; Klimach, T.; Konemann, T.; Kraemer, M.; Krüger, M. L.; Machado, L.; Mertes, S.; Pöhlker, C.; Poeschl, U.; Sauer, D. N.; Schnaiter, M.; Schneider, J.; Schulz, C.; Spanu, A.; Walser, A.; Weinzierl, B.; Wendisch, M.

2015-12-01

The German-Brazilian cooperative aircraft campaign ACRIDICON-CHUVA (Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems) on the German research aircraft HALO took place over the Amazon Basin in September/October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with trace gases, aerosol particles, and atmospheric radiation. The aircraft was equipped with about 30 remote sensing and in-situ instruments for meteorological, trace gas, aerosol, cloud, precipitation, and solar radiation measurements. Fourteen research flights were conducted during this campaign. Observations during ACRIDICON-CHUVA showed high aerosol concentrations in the upper troposphere (UT) over the Amazon Basin, with concentrations after normalization to standard conditions often exceeding those in the boundary layer (BL). This behavior was consistent between several aerosol metrics, including condensation nuclei (CN), cloud condensation nuclei (CCN), and chemical species mass concentrations. These UT aerosols were different in their composition and size distribution from the aerosol in the BL, making convective transport of particles unlikely as a source. The regions in the immediate outflow of deep convective clouds were found to be depleted in aerosol particles, whereas enhanced aerosol number and mass concentrations were found in UT regions that had experienced outflow from deep convection in the preceding 24-48 hours. This suggests that aerosol production takes place in the UT based on volatile and condensable material brought up by deep convection. Subsequently, downward mixing and transport of upper tropospheric aerosol may be a source of particles to the BL, where they increase in size by the condensation of biogenic volatile organic carbon (BVOC) oxidation products. This may be an important source of aerosol particles in the Amazonian BL, where aerosol nucleation and new particle formation has not been observed.

Application and Evaluation of an Explicit Prognostic Cloud-Cover Scheme in GRAPES Global Forecast System

NASA Astrophysics Data System (ADS)

Ma, Zhanshan; Liu, Qijun; Zhao, Chuanfeng; Shen, Xueshun; Wang, Yuan; Jiang, Jonathan H.; Li, Zhe; Yung, Yuk

2018-03-01

An explicit prognostic cloud-cover scheme (PROGCS) is implemented into the Global/Regional Assimilation and Prediction System (GRAPES) for global middle-range numerical weather predication system (GRAPES_GFS) to improve the model performance in simulating cloud cover and radiation. Unlike the previous diagnostic cloud-cover scheme (DIAGCS), PROGCS considers the formation and dissipation of cloud cover by physically connecting it to the cumulus convection and large-scale stratiform condensation processes. Our simulation results show that clouds in mid-high latitudes arise mainly from large-scale stratiform condensation processes, while cumulus convection and large-scale condensation processes jointly determine cloud cover in low latitudes. Compared with DIAGCS, PROGCS captures more consistent vertical distributions of cloud cover with the observations from Atmospheric Radiation Measurements (ARM) program at the Southern Great Plains (SGP) site and simulates more realistic diurnal cycle of marine stratocumulus with the ERA-Interim reanalysis data. The low, high, and total cloud covers that are determined via PROGCS appear to be more realistic than those simulated via DIAGCS when both are compared with satellite retrievals though the former maintains slight negative biases. In addition, the simulations of outgoing longwave radiation (OLR) at the top of the atmosphere (TOA) from PROGCS runs have been considerably improved as well, resulting in less biases in radiative heating rates at heights below 850 hPa and above 400 hPa of GRAPES_GFS. Our results indicate that a prognostic method of cloud-cover calculation has significant advantage over the conventional diagnostic one, and it should be adopted in both weather and climate simulation and forecast.

Massive superclusters as a probe of the nature and amplitude of primordial density fluctuations

NASA Technical Reports Server (NTRS)

Kaiser, N.; Davis, M.

1985-01-01

It is pointed out that correlation studies of galaxy positions have been widely used in the search for information about the large-scale matter distribution. The study of rare condensations on large scales provides an approach to extend the existing knowledge of large-scale structure into the weakly clustered regime. Shane (1975) provides a description of several apparent massive condensations within the Shane-Wirtanen catalog, taking into account the Serpens-Virgo cloud and the Corona cloud. In the present study, a description is given of a model for estimating the frequency of condensations which evolve from initially Gaussian fluctuations. This model is applied to the Corona cloud to estimate its 'rareness' and thereby estimate the rms density contrast on this mass scale. An attempt is made to find a conflict between the density fluctuations derived from the Corona cloud and independent constraints. A comparison is conducted of the estimate and the density fluctuations predicted to arise in a universe dominated by cold dark matter.

Cloud Condensation Nuclei in FIRE III

NASA Technical Reports Server (NTRS)

Hudson, James G.; Delnore, Victor E. (Technical Monitor)

2002-01-01

Yum and Hudson showed that the springtime Arctic aerosol is probably a result of long-range transport at high altitudes. Scavenging of particles by clouds reduces the low level concentrations by a factor of 3. This produces a vertical gradient in particle concentrations when low-level clouds are present. Concentrations are uniform with height when clouds are not present. Low-level CCN (cloud condensation nuclei) spectra are similar to those in other maritime areas as found by previous projects including FIRE 1 and ASTEX, which were also supported on earlier NASA-FIRE grants. Wylie and Hudson carried this work much further by comparing the CCN spectra observed during ACE with back trajectories of air masses and satellite photographs. This showed that cloud scavenging reduces CCN concentrations at all altitudes over the springtime Arctic, with liquid clouds being more efficient scavengers than frozen clouds. The small size of the Arctic Ocean seems to make it more susceptible to continental and thus anthropogenic aerosol influences than any of the other larger oceans.

Airborne measurements of cloud-forming nuclei and aerosol particles in stabilized ground clouds produced by solid rocket booster firings

NASA Technical Reports Server (NTRS)

Hindman, E. E., II; Ala, G. G.; Parungo, F. P.; Willis, P. T.; Bendura, R. J.; Woods, D.

1978-01-01

Airborne measurements of cloud volumes, ice nuclei and cloud condensation nuclei, liquid particles, and aerosol particles were obtained from stabilized ground clouds (SGCs) produced by Titan 3 launches at Kennedy Space Center, 20 August and 5 September 1977. The SGCs were bright, white, cumulus clouds early in their life and contained up to 3.5 g/m3 of liquid in micron to millimeter size droplets. The measured cloud volumes were 40 to 60 cu km five hours after launch. The SGCs contained high concentrations of cloud condensation nuclei active at 0.2%, 0.5%, and 1.0% supersaturation for periods of three to five hours. The SGCs also contained high concentrations of submicron particles. Three modes existed in the particle population: a 0.05 to 0.1 micron mode composed of aluminum-containing particles, a 0.2 to 0.8 micron mode, and a 2.0 to 10 micron mode composed of particles that contained primarily aluminum.

Aerosol impacts on deep convective storms in the tropics: A combination of modeling and observations

NASA Astrophysics Data System (ADS)

Storer, Rachel Lynn

It is widely accepted that increasing the number of aerosols available to act as cloud condensation nuclei (CCN) will have significant effects on cloud properties, both microphysical and dynamical. This work focuses on the impacts of aerosols on deep convective clouds (DCCs), which experience more complicated responses than warm clouds due to their strong dynamical forcing and the presence of ice processes. Several previous studies have seen that DCCs may be invigorated by increasing aerosols, though this is not the case in all scenarios. The precipitation response to increased aerosol concentrations is also mixed. Often precipitation is thought to decrease due to a less efficient warm rain process in polluted clouds, yet convective invigoration would lead to an overall increase in surface precipitation. In this work, modeling and observations are both used in order to enhance our understanding regarding the effects of aerosols on DCCs. Specifically, the area investigated is the tropical East Atlantic, where dust from the coast of Africa frequently is available to interact with convective storms over the ocean. The first study investigates the effects of aerosols on tropical DCCs through the use of numerical modeling. A series of large-scale, two-dimensional cloud-resolving model simulations was completed, differing only in the concentration of aerosols available to act as CCN. Polluted simulations contained more deep convective clouds, wider storms, higher cloud tops and more convective precipitation across the entire domain. Differences in the warm cloud microphysical processes were largely consistent with aerosol indirect theory, and the average precipitation produced in each DCC column decreased with increasing aerosol concentration. A detailed microphysical budget analysis showed that the reduction in collision and coalescence largely dominated the trend in surface precipitation; however the production of rain through the melting of ice, though it also decreased, became more important as the aerosol concentration increased. The DCCs in polluted simulations contained more frequent, stronger updrafts and downdrafts, but the average updraft speed decreased with increasing aerosols in DCCs above 6 km. An examination of the buoyancy term of the vertical velocity equation demonstrates that the drag associated with condensate loading is an important factor in determining the average updraft strength. The largest contributions to latent heating in DCCs were cloud nucleation and vapor deposition onto water and ice, but changes in latent heating were, on average, an order of magnitude smaller than those in the condensate loading term. It is suggested that the average updraft is largely influenced by condensate loading in the more extensive stratiform regions of the polluted storms, while invigoration in the convective core leads to stronger updrafts and higher cloud tops. The goal of the second study was to examine observational data for evidence that would support the findings of the modeling work. In order to do this, four years of CloudSat data were analyzed over a region of the East Atlantic, chosen for the similarity (in meteorology and the presence of aerosols) to the modeling study. The satellite data were combined with information about aerosols taken from the output of a global transport model, and only those profiles fitting the definition of deep convective clouds were analyzed. Overall, the cloud center of gravity, cloud top, rain top, and ice water path were all found to increase with increased aerosol loading. These findings are in agreement with what was found in the modeling work, and are suggestive of convective invigoration with increased aerosols. In order to separate environmental effects from that due to aerosols, the data were sorted by environmental convective available potential energy (CAPE) and lower tropospheric static stability (LTSS). The aerosol effects were found to be largely independent of the environment. A simple statistical test suggests that the difference between the cleanest and most polluted clouds sampled are significant, lending credence to the hypothesis of convective invigoration. This is the first time evidence of deep convective invigoration has been demonstrated within a large region and over a long time period, and it is quite promising that there are many similarities between the modeling and observational results.

Why do general circulation models overestimate the aerosol cloud lifetime effect? A case study comparing CAM5 and a CRM

NASA Astrophysics Data System (ADS)

Zhou, Cheng; Penner, Joyce E.

2017-01-01

Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water path (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 27 May 2011 at the southern Great Plains (SGP) measurement site established by the Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) program using a single-column version of a global climate model (Community Atmosphere Model or CAM) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP in CAM is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near the cloud top, resulting in an overall decrease in LWP. Our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.

Effects of aerosol from biomass burning on the global radiation budget

NASA Technical Reports Server (NTRS)

Penner, Joyce E.; Dickinson, Robert E.; O'Neill, Christine A.

1992-01-01

An analysis is made of the likely contribution of smoke particles from biomass burning to the global radiation balance. These particles act to reflect solar radiation directly; they also can act as cloud condensation nuclei, increasing the reflectivity of clouds. Together these effects, although uncertain, may add up globally to a cooling effect as large as 2 watts per square meter, comparable to the estimated contribution to sulfate aerosols. Anthropogenic increases of smoke emission thus may have helped weaken the net greenhouse warming from anthropogenic trace gases.

Evolution of the Far-Infrared Cloud at Titan's South Pole

NASA Technical Reports Server (NTRS)

Jennings, Donald E.; Achterberg, R. K.; Cottini, V.; Anderson, C. M.; Flasar, F. M.; Nixon, C. A.; Bjoraker, G. L.; Kunde, V. G.; Carlson, R. C.; Guandique, E.;

Aerosol effects on clouds and precipitation over the eastern China

NASA Astrophysics Data System (ADS)

Wang, W. C.; Chen, G.; Song, Y.

2017-12-01

Anthropogenic aerosols (sulfates, nitrates and black carbons) can act as cloud condensation nuclei to regulate cloud droplet number and size, thereby changing cloud radiative properties and atmospheric short- and long-wave radiation. These together with aerosol direct radiative effects in turn alter the circulation with likely effects on the spatial distribution of cloud and precipitation. We conduct WRF model simulations over the eastern China to investigate the aerosol-cloud-climate interactions. In general, more aerosols yield more but smaller cloud droplets and larger cloud water content, whereas the changes of vertical distribution of cloud cover exhibit strong regional variations. For example, the low-cloud fraction and water content increase by more than 10% over the west part of the Yangtze-Huai River Valley (YHRV) and the southeast coastal region, but decrease over the east part of the YHRV, and high-cloud fraction decreases in South and North China but increases in the YHRV. The radiative forcing of aerosols and cloud changes are compared, with focus on the effects of changes of vertical distribution of cloud properties (microphysics and fraction). The precipitation changes are found to be closely associated with the circulation change, which favors more (and longer duration) rainfall over the YHRV but less (and shorter) rainfall over other regions. Details of the circulation change and its associations with clouds and precipitation will be presented.

Implementation of warm-cloud processes in a source-oriented WRF/Chem model to study the effect of aerosol mixing state on fog formation in the Central Valley of California

NASA Astrophysics Data System (ADS)

Lee, Hsiang-He; Chen, Shu-Hua; Kleeman, Michael J.; Zhang, Hongliang; DeNero, Steven P.; Joe, David K.

2016-07-01

The source-oriented Weather Research and Forecasting chemistry model (SOWC) was modified to include warm cloud processes and was applied to investigate how aerosol mixing states influence fog formation and optical properties in the atmosphere. SOWC tracks a 6-D chemical variable (X, Z, Y, size bins, source types, species) through an explicit simulation of atmospheric chemistry and physics. A source-oriented cloud condensation nuclei module was implemented into the SOWC model to simulate warm clouds using the modified two-moment Purdue Lin microphysics scheme. The Goddard shortwave and long-wave radiation schemes were modified to interact with source-oriented aerosols and cloud droplets so that aerosol direct and indirect effects could be studied. The enhanced SOWC model was applied to study a fog event that occurred on 17 January 2011, in the Central Valley of California. Tule fog occurred because an atmospheric river effectively advected high moisture into the Central Valley and nighttime drainage flow brought cold air from mountains into the valley. The SOWC model produced reasonable liquid water path, spatial distribution and duration of fog events. The inclusion of aerosol-radiation interaction only slightly modified simulation results since cloud optical thickness dominated the radiation budget in fog events. The source-oriented mixture representation of particles reduced cloud droplet number relative to the internal mixture approach that artificially coats hydrophobic particles with hygroscopic components. The fraction of aerosols activating into cloud condensation nuclei (CCN) at a supersaturation of 0.5 % in the Central Valley decreased from 94 % in the internal mixture model to 80 % in the source-oriented model. This increased surface energy flux by 3-5 W m-2 and surface temperature by as much as 0.25 K in the daytime.

Quantum Enhancement of the Index of Refraction in a Bose-Einstein Condensate.

PubMed

Bons, P C; de Haas, R; de Jong, D; Groot, A; van der Straten, P

2016-04-29

We study the index of refraction of an ultracold bosonic gas in the dilute regime. Using phase-contrast imaging with light detuned from resonance by several tens of linewidths, we image a single cloud of ultracold atoms for 100 consecutive shots, which enables the study of the scattering rate as a function of temperature and density using only a single cloud. We observe that the scattering rate is increased below the critical temperature for Bose-Einstein condensation by a factor of 3 compared to the single-atom scattering rate. We show that current atom-light interaction models to second order of the density show a similar increase, where the magnitude of the effect depends on the model that is used to calculate the pair-correlation function. This confirms that the effect of quantum statistics on the index of refraction is dominant in this regime.

Numerical Simulation of an Industrial Cumulus Affected by Heat, Moisture, and CCN Released from an Oil Refinery.

NASA Astrophysics Data System (ADS)

Guan, S.; Reuter, G. W.

1996-08-01

Large oil refineries emit heat, vapor, and cloud condensation nuclei (CCN), all of which can affect the formation of cloud and precipitation. This study quantities the relative contributions of the three factors on cloud development in calm wind conditions using an axisymmetric cloud model. The factor separation technique is applied to isolate the net contributions of waste heat, vapor, and CCN on the rainfall of a cumulus developing in the industrial plume. The mutual-interactive contributions of two or three of the factors are also computed.The simulations for midlatitude and tropical conditions indicate that the sensible heat provides the major stimulus for cloud development and rain formation. The pure contribution of the industrial CCN is to enhance the condensation, causing an increase in the mass of total cloud water. The simulation results indicate that mutual interactions between waste heat and industrial CCN are large for both cases considered.

Large Scale Ice Water Path and 3-D Ice Water Content

DOE Data Explorer

Liu, Guosheng

2008-01-15

Cloud ice water concentration is one of the most important, yet poorly observed, cloud properties. Developing physical parameterizations used in general circulation models through single-column modeling is one of the key foci of the ARM program. In addition to the vertical profiles of temperature, water vapor and condensed water at the model grids, large-scale horizontal advective tendencies of these variables are also required as forcing terms in the single-column models. Observed horizontal advection of condensed water has not been available because the radar/lidar/radiometer observations at the ARM site are single-point measurement, therefore, do not provide horizontal distribution of condensed water. The intention of this product is to provide large-scale distribution of cloud ice water by merging available surface and satellite measurements. The satellite cloud ice water algorithm uses ARM ground-based measurements as baseline, produces datasets for 3-D cloud ice water distributions in a 10 deg x 10 deg area near ARM site. The approach of the study is to expand a (surface) point measurement to an (satellite) areal measurement. That is, this study takes the advantage of the high quality cloud measurements at the point of ARM site. We use the cloud characteristics derived from the point measurement to guide/constrain satellite retrieval, then use the satellite algorithm to derive the cloud ice water distributions within an area, i.e., 10 deg x 10 deg centered at ARM site.

Allowing for Horizontally Heterogeneous Clouds and Generalized Overlap in an Atmospheric GCM

NASA Technical Reports Server (NTRS)

Lee, D.; Oreopoulos, L.; Suarez, M.

2011-01-01

While fully accounting for 3D effects in Global Climate Models (GCMs) appears not realistic at the present time for a variety of reasons such as computational cost and unavailability of 3D cloud structure in the models, incorporation in radiation schemes of subgrid cloud variability described by one-point statistics is now considered feasible and is being actively pursued. This development has gained momentum once it was demonstrated that CPU-intensive spectrally explicit Independent Column Approximation (lCA) can be substituted by stochastic Monte Carlo ICA (McICA) calculations where spectral integration is accomplished in a manner that produces relatively benign random noise. The McICA approach has been implemented in Goddard's GEOS-5 atmospheric GCM as part of the implementation of the RRTMG radiation package. GEOS-5 with McICA and RRTMG can handle horizontally variable clouds which can be set via a cloud generator to arbitrarily overlap within the full spectrum of maximum and random both in terms of cloud fraction and layer condensate distributions. In our presentation we will show radiative and other impacts of the combined horizontal and vertical cloud variability on multi-year simulations of an otherwise untuned GEOS-5 with fixed SSTs. Introducing cloud horizontal heterogeneity without changing the mean amounts of condensate reduces reflected solar and increases thermal radiation to space, but disproportionate changes may increase the radiative imbalance at TOA. The net radiation at TOA can be modulated by allowing the parameters of the generalized overlap and heterogeneity scheme to vary, a dependence whose behavior we will discuss. The sensitivity of the cloud radiative forcing to the parameters of cloud horizontal heterogeneity and comparisons of CERES-derived forcing will be shown.

Planetary atmospheres program

NASA Technical Reports Server (NTRS)

1982-01-01

Chemical and physical models of the Jovian subnebula are addressed. Halide cloud condensation and volatile element inventories on Venus and considered. Computation methods for isolated grain condensation behavior are examined.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bae, Soo Ya; Jeong, Jaein I.; Park, R.

We examine the effect of anthropogenic aerosols on the weekly variability of precipitation in Korea in summer 2004 by using Weather Research and Forecasting (WRF) and Community Multiscale Air Quality (CMAQ) models. We con-duct two WRF simulations including a baseline simulation with empirically based cloud condensation nuclei (CCN) number concentrations and a sensitivity simulation with our implementation to account for the effect of aerosols on CCN number concentrations. The first simulation underestimates observed precipitation amounts, particularly in northeastern coastal areas of Korea, whereas the latter shows higher precipitation amounts that are in better agree-ment with the observations. In addition, themore » sensitivity model with the aerosol effects reproduces the observed weekly variability, particularly for precipitation frequency with a high R at 0.85, showing 20% increase of precipita-tion events during the weekend than those during weekdays. We find that the aerosol effect results in higher CCN number concentrations during the weekdays and a three-fold increase of the cloud water mixing ratio through en-hanced condensation. As a result, the amount of warm rain is generally suppressed because of the low auto-conversion process from cloud water to rain water under high aerosol conditions. The inefficient conversion, how-ever, leads to higher vertical development of clouds in the mid-atmosphere with stronger updrafts in the sensitivity model, which increases by 21% cold-phase hydrometeors including ice, snow, and graupel relative to the baseline model and ultimately results in higher precipitation amounts in summer.« less

Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin

NASA Astrophysics Data System (ADS)

Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel; Amorim Holanda, Bruna; Artaxo, Paulo; Barbosa, Henrique M. J.; Borrmann, Stephan; Cecchini, Micael A.; Costa, Anja; Dollner, Maximilian; Fütterer, Daniel; Järvinen, Emma; Jurkat, Tina; Klimach, Thomas; Konemann, Tobias; Knote, Christoph; Krämer, Martina; Krisna, Trismono; Machado, Luiz A. T.; Mertes, Stephan; Minikin, Andreas; Pöhlker, Christopher; Pöhlker, Mira L.; Pöschl, Ulrich; Rosenfeld, Daniel; Sauer, Daniel; Schlager, Hans; Schnaiter, Martin; Schneider, Johannes; Schulz, Christiane; Spanu, Antonio; Sperling, Vinicius B.; Voigt, Christiane; Walser, Adrian; Wang, Jian; Weinzierl, Bernadett; Wendisch, Manfred; Ziereis, Helmut

2018-01-01

Airborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15 km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German-Brazilian cooperative aircraft campaign ACRIDICON-CHUVA, where ACRIDICON stands for Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems and CHUVA is the acronym for Cloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (global precipitation measurement), on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September-October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation. Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles (< 90 nm diameter) were found in UT regions that had experienced outflow from deep convection in the preceding 5-72 h. We also found elevated concentrations of larger (> 90 nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN. Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol can be a source of particles to the PBL, where they increase in size by the condensation of biogenic volatile organic compound (BVOC) oxidation products. This may be an important source of aerosol particles for the Amazonian PBL, where aerosol nucleation and new particle formation have not been observed. We propose that this may have been the dominant process supplying secondary aerosol particles in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles.

Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin

DOE PAGES

Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel; ...

2018-01-25

Airborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15 km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German–Brazilian cooperative aircraft campaign ACRIDICON–CHUVA, where ACRIDICON stands for Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems and CHUVA is the acronym for Cloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (globalmore » precipitation measurement), on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September–October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation. Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles (< 90 nm diameter) were found in UT regions that had experienced outflow from deep convection in the preceding 5–72 h. We also found elevated concentrations of larger (> 90 nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN. Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol can be a source of particles to the PBL, where they increase in size by the condensation of biogenic volatile organic compound (BVOC) oxidation products. This may be an important source of aerosol particles for the Amazonian PBL, where aerosol nucleation and new particle formation have not been observed. We propose that this may have been the dominant process supplying secondary aerosol particles in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles.« less

Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin

DOE Office of Scientific and Technical Information (OSTI.GOV)

Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel

Airborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15 km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German–Brazilian cooperative aircraft campaign ACRIDICON–CHUVA, where ACRIDICON stands for Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems and CHUVA is the acronym for Cloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (globalmore » precipitation measurement), on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September–October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation. Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles (< 90 nm diameter) were found in UT regions that had experienced outflow from deep convection in the preceding 5–72 h. We also found elevated concentrations of larger (> 90 nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN. Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol can be a source of particles to the PBL, where they increase in size by the condensation of biogenic volatile organic compound (BVOC) oxidation products. This may be an important source of aerosol particles for the Amazonian PBL, where aerosol nucleation and new particle formation have not been observed. We propose that this may have been the dominant process supplying secondary aerosol particles in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles.« less

Modeling the Impact of Drizzle and 3D Cloud Structure on Remote Sensing of Effective Radius

NASA Technical Reports Server (NTRS)

Platnick, Steven; Zinner, Tobias; Ackerman, S.

2008-01-01

Remote sensing of cloud particle size with passive sensors like MODIS is an important tool for cloud microphysical studies. As a measure of the radiatively relevant droplet size, effective radius can be retrieved with different combinations of visible through shortwave infrared channels. MODIS observations sometimes show significantly larger effective radii in marine boundary layer cloud fields derived from the 1.6 and 2.1 pm channel observations than for 3.7 pm retrievals. Possible explanations range from 3D radiative transport effects and sub-pixel cloud inhomogeneity to the impact of drizzle formation on the droplet distribution. To investigate the potential influence of these factors, we use LES boundary layer cloud simulations in combination with 3D Monte Carlo simulations of MODIS observations. LES simulations of warm cloud spectral microphysics for cases of marine stratus and broken stratocumulus, each for two different values of cloud condensation nuclei density, produce cloud structures comprising droplet size distributions with and without drizzle size drops. In this study, synthetic MODIS observations generated from 3D radiative transport simulations that consider the full droplet size distribution will be generated for each scene. The operational MODIS effective radius retrievals will then be applied to the simulated reflectances and the results compared with the LES microphysics.

Surfactants from the gas phase may promote cloud droplet formation.

PubMed

Sareen, Neha; Schwier, Allison N; Lathem, Terry L; Nenes, Athanasios; McNeill, V Faye

2013-02-19

Clouds, a key component of the climate system, form when water vapor condenses upon atmospheric particulates termed cloud condensation nuclei (CCN). Variations in CCN concentrations can profoundly impact cloud properties, with important effects on local and global climate. Organic matter constitutes a significant fraction of tropospheric aerosol mass, and can influence CCN activity by depressing surface tension, contributing solute, and influencing droplet activation kinetics by forming a barrier to water uptake. We present direct evidence that two ubiquitous atmospheric trace gases, methylglyoxal (MG) and acetaldehyde, known to be surface-active, can enhance aerosol CCN activity upon uptake. This effect is demonstrated by exposing acidified ammonium sulfate particles to 250 parts per billion (ppb) or 8 ppb gas-phase MG and/or acetaldehyde in an aerosol reaction chamber for up to 5 h. For the more atmospherically relevant experiments, i.e., the 8-ppb organic precursor concentrations, significant enhancements in CCN activity, up to 7.5% reduction in critical dry diameter for activation, are observed over a timescale of hours, without any detectable limitation in activation kinetics. This reduction in critical diameter enhances the apparent particle hygroscopicity up to 26%, which for ambient aerosol would lead to cloud droplet number concentration increases of 8-10% on average. The observed enhancements exceed what would be expected based on Köhler theory and bulk properties. Therefore, the effect may be attributed to the adsorption of MG and acetaldehyde to the gas-aerosol interface, leading to surface tension depression of the aerosol. We conclude that gas-phase surfactants may enhance CCN activity in the atmosphere.

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

NASA Technical Reports Server (NTRS)

Tao, Wei-Kuo; Li, X.; Khain, A.; Simpson, S.

2005-01-01

Cloud microphysics are inevitable affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds, Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effect of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, a detailed spectral-bin microphysical scheme was implemented into the the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bim microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.

Simulation of Asia Dust and Cloud Interaction Over Pacific Ocean During Pacdex

NASA Astrophysics Data System (ADS)

Long, X.; Huang, J.; Cheng, C.; Wang, W.

2007-12-01

The effect of dust plume on the Pacific cloud systems and the associated radiative forcing is an outstanding problem for understanding climate change. Many studies showing that dust aerosol might be a good absorber for solar radiation, at the same time dust aerosols could affect the cloud's formation and precipitation by its capability as cloud condensation nuclei (CCN) and ice forming nuclei (IFN). But the role of aerosols in clouds and precipitation is very complex. Simulation of interaction between cloud and dust aerosols requires recognition that the aerosol cloud system comprises coupled components of dynamics, aerosol and cloud microphysics, radiation processes. In this study, we investigated the interaction between dust aerosols and cloud with WRF which coupled with detailed cloud microphysics processes and dust process. The observed data of SACOL (Semi-Arid Climate and Environment Observatory of Lanzhou University) and PACDEX (Pacific Dust Experiment) is used as the initialization which include the vertical distributions and concentration of dust particles. Our results show that dust aerosol not only impacts cloud microphysical processes but also cloud microstructure; Dust aerosols can act as effective ice nuclei and intensify the ice-forming processes.

Chinese SO2 pollution over Europe - Part 2: Simulation of aerosol and cloud condensation nuclei formation

NASA Astrophysics Data System (ADS)

Fiedler, V.; Arnold, F.; Schlager, H.; Pirjola, L.

2009-01-01

We report on sulfur dioxide (SO2) induced formation of aerosols and cloud condensation nuclei in an SO2 rich aged (9 days) pollution plume of Chinese origin, which we have detected at 5-7 km altitude during a research aircraft mission over the East Atlantic off the West coast of Ireland. Building on our measurements of SO2 and other trace gases along with plume trajectory simulations, we have performed model simulations of SO2 induced formation of gaseous sulfuric acid (GSA, H2SO4) followed by GSA induced formation and growth of aerosol particles. We find that efficient photochemical SO2 conversion to GSA took place in the plume followed by efficient formation and growth of H2SO4-H2O aerosol particles. Most particles reached sufficiently large sizes to act as cloud condensation nuclei whenever water vapor supersaturation exceeded 0.1-0.2%. As a consequence, smaller but more numerous cloud droplets are formed, which tend to increase the cloud albedo and to decrease the rainout efficiency. The detected plume represents an interesting example of the environmental impact of long range transport of fossil fuel combustion generated SO2.

CHASER: An Innovative Satellite Mission Concept to Measure the Effects of Aerosols on Clouds and Climate

NASA Astrophysics Data System (ADS)

Renno, N.; Williams, E.; Rosenfeld, D.; Fischer, D.; Fischer, J.; Kremic, T.; Agrawal, A.; Andreae, M.; Bierbaum, R.; Blakeslee, R.; Boerner, A.; Bowles, N.; Christian, H.; Dunion, J.; Horvath, A.; Huang, X.; Khain, A.; Kinne, S.; Lemos, M.-C.; Penner, J.

2012-04-01

The formation of cloud droplets on aerosol particles, technically known as the activation of cloud condensation nuclei (CCN), is the fundamental process driving the interactions of aerosols with clouds and precipitation. Knowledge of these interactions is foundational to our understanding of weather and climate. The Intergovernmental Panel on Climate Change (IPCC) and the Decadal Survey (NRC 2007) indicate that the uncertainty in how clouds adjust to aerosol perturbations dominates the uncertainty in the overall quantification of the radiative forcing attributable to human activities. The Clouds, Hazards, and Aerosols Survey for Earth Researchers (CHASER) mission concept responds to the IPCC and Decadal Survey concerns by studying the activation of CCN and their interactions with clouds and storms. CHASER proposes to revolutionize our understanding of the interactions of aerosols with clouds by making the first global measurements of the fundamental physical entity linking them: activated cloud condensation nuclei. The CHASER mission was conceptualized to measure all quantities necessary for determining the interactions of aerosols with clouds and storms. Measurements by current satellites allow the determination of crude profiles of cloud particle size but not of the activated CCN that seed them. CHASER uses a new technique (Freud et al. 2011; Rosenfeld et al. 2012) and high-heritage instruments to produce the first global maps of activated CCN and the properties of the clouds associated with them. CHASER measures the CCN concentration and cloud thermodynamic forcing simultaneously, allowing their effects to be distinguished. Changes in the behavior of a group of weather systems in which only one of the quantities varies (a partial derivative of the intensity with the desirable quantity) allow the determination of each effect statistically. The high uncertainties of current climate predictions limit their much-needed use in decision-making. CHASER mitigates this problem by establishing a Data Application Center for conducting social science research focused on understanding the best ways to use, transfer, and communicate mission data to decision-makers. The CHASER Data Application Center supports the visions of the National Research Council and the Decadal Survey for an integrated program of observations from space that secures practical benefits for humankind by developing data products for assessing risks due to severe weather and climate change.

Planetary atmospheres program

NASA Technical Reports Server (NTRS)

1982-01-01

Non-solar compositional models of the troposphere of Jupiter, halide cloud condensation and volatile element inventories on Venus, and shock-wave processing of interstellar cloud materials are discussed.

Aerosol effect on the evolution of the thermodynamic properties of warm convective cloud fields

PubMed Central

Dagan, Guy; Koren, Ilan; Altaratz, Orit; Heiblum, Reuven H.

2016-01-01

Convective cloud formation and evolution strongly depend on environmental temperature and humidity profiles. The forming clouds change the profiles that created them by redistributing heat and moisture. Here we show that the evolution of the field’s thermodynamic properties depends heavily on the concentration of aerosol, liquid or solid particles suspended in the atmosphere. Under polluted conditions, rain formation is suppressed and the non-precipitating clouds act to warm the lower part of the cloudy layer (where there is net condensation) and cool and moisten the upper part of the cloudy layer (where there is net evaporation), thereby destabilizing the layer. Under clean conditions, precipitation causes net warming of the cloudy layer and net cooling of the sub-cloud layer (driven by rain evaporation), which together act to stabilize the atmosphere with time. Previous studies have examined different aspects of the effects of clouds on their environment. Here, we offer a complete analysis of the cloudy atmosphere, spanning the aerosol effect from instability-consumption to enhancement, below, inside and above warm clouds, showing the temporal evolution of the effects. We propose a direct measure for the magnitude and sign of the aerosol effect on thermodynamic instability. PMID:27929097

Aerosol effect on the evolution of the thermodynamic properties of warm convective cloud fields.

PubMed

Dagan, Guy; Koren, Ilan; Altaratz, Orit; Heiblum, Reuven H

2016-12-08

Convective cloud formation and evolution strongly depend on environmental temperature and humidity profiles. The forming clouds change the profiles that created them by redistributing heat and moisture. Here we show that the evolution of the field's thermodynamic properties depends heavily on the concentration of aerosol, liquid or solid particles suspended in the atmosphere. Under polluted conditions, rain formation is suppressed and the non-precipitating clouds act to warm the lower part of the cloudy layer (where there is net condensation) and cool and moisten the upper part of the cloudy layer (where there is net evaporation), thereby destabilizing the layer. Under clean conditions, precipitation causes net warming of the cloudy layer and net cooling of the sub-cloud layer (driven by rain evaporation), which together act to stabilize the atmosphere with time. Previous studies have examined different aspects of the effects of clouds on their environment. Here, we offer a complete analysis of the cloudy atmosphere, spanning the aerosol effect from instability-consumption to enhancement, below, inside and above warm clouds, showing the temporal evolution of the effects. We propose a direct measure for the magnitude and sign of the aerosol effect on thermodynamic instability.

Corona discharge induced snow formation in a cloud chamber.

PubMed

Ju, Jingjing; Wang, Tie-Jun; Li, Ruxin; Du, Shengzhe; Sun, Haiyi; Liu, Yonghong; Tian, Ye; Bai, Yafeng; Liu, Yaoxiang; Chen, Na; Wang, Jingwei; Wang, Cheng; Liu, Jiansheng; Chin, S L; Xu, Zhizhan

2017-09-18

Artificial rainmaking is in strong demand especially in arid regions. Traditional methods of seeding various Cloud Condensation Nuclei (CCN) into the clouds are costly and not environment friendly. Possible solutions based on ionization were proposed more than 100 years ago but there is still a lack of convincing verification or evidence. In this report, we demonstrated for the first time the condensation and precipitation (or snowfall) induced by a corona discharge inside a cloud chamber. Ionic wind was found to have played a more significant role than ions as extra CCN. In comparison with another newly emerging femtosecond laser filamentation ionization method, the snow precipitation induced by the corona discharge has about 4 orders of magnitude higher wall-plug efficiency under similar conditions.

A photoionization model for the optical line emission from cooling flows

NASA Technical Reports Server (NTRS)

Donahue, Megan; Voit, G. M.

1991-01-01

The detailed predictions of a photoionization model previously outlined in Voit and Donahue (1990) to explain the optical line emission associated with cooling flows in X-ray emitting clusters of galaxies are presented. In this model, EUV/soft X-ray radiation from condensing gas photoionizes clouds that have already cooled. The energetics and specific consequences of such a model, as compared to other models put forth in the literature is discussed. Also discussed are the consequences of magnetic fields and cloud-cloud shielding. The results illustrate how varying the individual column densities of the ionized clouds can reproduce the range of line ratios observed and strongly suggest that the emission-line nebulae are self-irradiated condensing regions at the centers of cooling flows.

Boreal forests, aerosols and the impacts on clouds and climate.

PubMed

Spracklen, Dominick V; Bonn, Boris; Carslaw, Kenneth S

2008-12-28

Previous studies have concluded that boreal forests warm the climate because the cooling from storage of carbon in vegetation and soils is cancelled out by the warming due to the absorption of the Sun's heat by the dark forest canopy. However, these studies ignored the impacts of forests on atmospheric aerosol. We use a global atmospheric model to show that, through emission of organic vapours and the resulting condensational growth of newly formed particles, boreal forests double regional cloud condensation nuclei concentrations (from approx. 100 to approx. 200 cm(-3)). Using a simple radiative model, we estimate that the resulting change in cloud albedo causes a radiative forcing of between -1.8 and -6.7 W m(-2) of forest. This forcing may be sufficiently large to result in boreal forests having an overall cooling impact on climate. We propose that the combination of climate forcings related to boreal forests may result in an important global homeostasis. In cold climatic conditions, the snow-vegetation albedo effect dominates and boreal forests warm the climate, whereas in warmer climates they may emit sufficiently large amounts of organic vapour modifying cloud albedo and acting to cool climate.

Implementation of aerosol-cloud interactions in the regional atmosphere-aerosol model COSMO-MUSCAT(5.0) and evaluation using satellite data

NASA Astrophysics Data System (ADS)

Dipu, Sudhakar; Quaas, Johannes; Wolke, Ralf; Stoll, Jens; Mühlbauer, Andreas; Sourdeval, Odran; Salzmann, Marc; Heinold, Bernd; Tegen, Ina

2017-06-01

The regional atmospheric model Consortium for Small-scale Modeling (COSMO) coupled to the Multi-Scale Chemistry Aerosol Transport model (MUSCAT) is extended in this work to represent aerosol-cloud interactions. Previously, only one-way interactions (scavenging of aerosol and in-cloud chemistry) and aerosol-radiation interactions were included in this model. The new version allows for a microphysical aerosol effect on clouds. For this, we use the optional two-moment cloud microphysical scheme in COSMO and the online-computed aerosol information for cloud condensation nuclei concentrations (Cccn), replacing the constant Cccn profile. In the radiation scheme, we have implemented a droplet-size-dependent cloud optical depth, allowing now for aerosol-cloud-radiation interactions. To evaluate the models with satellite data, the Cloud Feedback Model Intercomparison Project Observation Simulator Package (COSP) has been implemented. A case study has been carried out to understand the effects of the modifications, where the modified modeling system is applied over the European domain with a horizontal resolution of 0.25° × 0.25°. To reduce the complexity in aerosol-cloud interactions, only warm-phase clouds are considered. We found that the online-coupled aerosol introduces significant changes for some cloud microphysical properties. The cloud effective radius shows an increase of 9.5 %, and the cloud droplet number concentration is reduced by 21.5 %.

Estimation of the Cloud condensation nuclei concentration(CCN) and aerosol optical depth(AOD) relation in the Arctic region

NASA Astrophysics Data System (ADS)

Jung, C. H.; Yoon, Y. J.; Ahn, S. H.; Kang, H. J.; Gim, Y. T.; Lee, B. Y.

2017-12-01

Information of the spatial and temporal variations of cloud condensation nuclei (CCN) concentrations is important in estimating aerosol indirect effects. Generally, CCN aerosol is difficult to estimate using remote sensing methods. Although there are many CCN measurements data, extensive measurements of CCN are not feasible because of the complex nature of the operation and high cost, especially in the Arctic region. Thus, there have been many attempts to estimate CCN concentrations from more easily obtainable parameters such as aerosol optical depth (AOD) because AOD has the advantage of being readily observed by remote sensing from space by several sensors. For example, some form of correlation was derived between AOD and the number concentration of cloud condensation nuclei (CCN) through the comparison results from AERONET network and CCN measurements (Andreae 2009). In this study, a parameterization of CCN concentration as a function of AOD at 500 nm is given in the Arctic region. CCN data was collected during the period 2007-2013 at the Zeppelin observatory (78.91° N, 11.89° E, 474 masl). The AERONET network and MODIS AOD data are compared with ground measured CCN measurement and the relations between AOD and CCN are parameterized. The seasonal characteristics as well as long term trends are also considered. Through the measurement, CCN concentration remains high during spring because of aerosol transportation from the mid-latitudes, known as Arctic Haze. Lowest CCN number densities were observed during Arctic autumn and early winter when aerosol long-range transport into the Arctic is not effective and new particle formation ceases. The results show that the relation between AOD and CCN shows a different parameter depending on the seasonal aerosol and CCN characteristics. This seasonal different CCN-AOD relation can be interpreted as many physico-chemical aerosol properties including aerosol size distribution, composition. ReferenceAndreae, M. O. (2009) Correlation between cloud condensation nuclei concentration and aerosol optical thickness in remote and polluted regions,2009, Atmos. Chem. Phys., 9, 543-556.

Aerosol microphysical and radiative effects on continental cloud ensembles

NASA Astrophysics Data System (ADS)

Wang, Yuan; Vogel, Jonathan M.; Lin, Yun; Pan, Bowen; Hu, Jiaxi; Liu, Yangang; Dong, Xiquan; Jiang, Jonathan H.; Yung, Yuk L.; Zhang, Renyi

2018-02-01

Aerosol-cloud-radiation interactions represent one of the largest uncertainties in the current climate assessment. Much of the complexity arises from the non-monotonic responses of clouds, precipitation and radiative fluxes to aerosol perturbations under various meteorological conditions. In this study, an aerosol-aware WRF model is used to investigate the microphysical and radiative effects of aerosols in three weather systems during the March 2000 Cloud Intensive Observational Period campaign at the US Southern Great Plains. Three simulated cloud ensembles include a low-pressure deep convective cloud system, a collection of less-precipitating stratus and shallow cumulus, and a cold frontal passage. The WRF simulations are evaluated by several ground-based measurements. The microphysical properties of cloud hydrometeors, such as their mass and number concentrations, generally show monotonic trends as a function of cloud condensation nuclei concentrations. Aerosol radiative effects do not influence the trends of cloud microphysics, except for the stratus and shallow cumulus cases where aerosol semi-direct effects are identified. The precipitation changes by aerosols vary with the cloud types and their evolving stages, with a prominent aerosol invigoration effect and associated enhanced precipitation from the convective sources. The simulated aerosol direct effect suppresses precipitation in all three cases but does not overturn the aerosol indirect effect. Cloud fraction exhibits much smaller sensitivity (typically less than 2%) to aerosol perturbations, and the responses vary with aerosol concentrations and cloud regimes. The surface shortwave radiation shows a monotonic decrease by increasing aerosols, while the magnitude of the decrease depends on the cloud type.

Simulation of the Upper Clouds and Hazes of Venus Using a Microphysical Cloud Model

NASA Astrophysics Data System (ADS)

McGouldrick, K.

2012-12-01

Several different microphysical and chemical models of the clouds of Venus have been developed in attempts to reproduce the in situ observations of the Venus clouds made by Pioneer Venus, Venera, and Vega descent probes (Turco et al., 1983 (Icarus 53:18-25), James et al, 1997 (Icarus 129:147-171), Imamura and Hashimoto, 2001 (J. Atm. Sci. 58:3597-3612), and McGouldrick and Toon, 2007 (Icarus 191:1-24)). The model of McGouldrick and Toon has successfully reproduced observations within the condensational middle and lower cloud decks of Venus (between about 48 and 57 km altitude, experiencing conditions similar to Earth's troposphere) and it now being extended to also simulate the microphysics occurring in the upper cloud deck (between altitudes of about 57 km and 70 km, experiencing conditions similar to Earth's stratosphere). In the upper clouds, aerosols composed of a solution of sulfuric acid in water are generated from the reservoir of available water vapor and sulfuric acid vapor that is photochemically produced. The manner of particle creation (e.g., activation of cloud condensation nuclei, or homogeneous or heterogeneous nucleation) is still incompletely understood, and the atmospheric environment has been measured to be not inconsistent with frozen aerosol particles (either sulfuric acid monohydrate or water ice). The material phase, viscosity, and surface tension of the aerosols (which are strongly dependent up on the local temperature and water vapor concentration) can affect the coagulation efficiencies of the aerosol, leading to variations in the size distributions, and other microphysical and radiative properties. Here, I present recent work exploring the effects of nucleation rates and coalescence efficiencies on the simulated Venus upper clouds.

Ozone, dust, smoke and humidity in nuclear winter

NASA Technical Reports Server (NTRS)

Turco, R. P.; Toon, O. B.; Ackerman, T. P.; Pollack, J. B.; Sagan, C.

1985-01-01

Recent correspondence on nuclear winter is commented on. Reasons are given for why the Tunguska meteor explosion may not be useful in calibrating the effects of a major nuclear exchange. The relationship between the optical depth of an aerosol cloud, the composition of the cloud, and its effect on sunlight intensity and climate are clarified. The significance of the Tambora eruption of 1815 and of historical fires for the nuclear winter theory are briefly discussed. The dispersion of smoke plumes from large fires is addressed, and water condensation and smoke scavenging are considered.

Cloud Condensation Nuclei Prediction Error from Application of Kohler Theory: Importance for the Aerosol Indirect Effect

NASA Technical Reports Server (NTRS)

Sotiropoulou, Rafaella-Eleni P.; Nenes, Athanasios; Adams, Peter J.; Seinfeld, John H.

2007-01-01

In situ observations of aerosol and cloud condensation nuclei (CCN) and the GISS GCM Model II' with an online aerosol simulation and explicit aerosol-cloud interactions are used to quantify the uncertainty in radiative forcing and autoconversion rate from application of Kohler theory. Simulations suggest that application of Koehler theory introduces a 10-20% uncertainty in global average indirect forcing and 2-11% uncertainty in autoconversion. Regionally, the uncertainty in indirect forcing ranges between 10-20%, and 5-50% for autoconversion. These results are insensitive to the range of updraft velocity and water vapor uptake coefficient considered. This study suggests that Koehler theory (as implemented in climate models) is not a significant source of uncertainty for aerosol indirect forcing but can be substantial for assessments of aerosol effects on the hydrological cycle in climatically sensitive regions of the globe. This implies that improvements in the representation of GCM subgrid processes and aerosol size distribution will mostly benefit indirect forcing assessments. Predictions of autoconversion, by nature, will be subject to considerable uncertainty; its reduction may require explicit representation of size-resolved aerosol composition and mixing state.

Storm clouds on Saturn: Lightning-induced chemistry and associated materials consistent with Cassini/VIMS spectra

USGS Publications Warehouse

Baines, K.H.; Delitsky, M.L.; Momary, T.W.; Brown, R.H.; Buratti, B.J.; Clark, R.N.; Nicholson, P.D.

2009-01-01

Thunderstorm activity on Saturn is associated with optically detectable clouds that are atypically dark throughout the near-infrared. As observed by Cassini/VIMS, these clouds are ~20% less reflective than typical neighboring clouds throughout the spectral range from 0.8 ??m to at least 4.1 ??m. We propose that active thunderstorms originating in the 10-20 bar water-condensation region vertically transport dark materials at depth to the ~1 bar level where they can be observed. These materials in part may be produced by chemical processes associated with lightning, likely within the water clouds near the ~10 bar freezing level of water, as detected by the electrostatic discharge of lightning flashes observed by Cassini/RPWS (e.g., Fischer et al. 2008, Space Sci. Rev., 137, 271-285). We review lightning-induced pyrolytic chemistry involving a variety of Saturnian constituents, including hydrogen, methane, ammonia, hydrogen sulfide, phosphine, and water. We find that the lack of absorption in the 1-2 ??m spectral region by lightning-generated sulfuric and phosphorous condensates renders these constituents as minor players in determining the color of the dark storm clouds. Relatively small particulates of elemental carbon, formed by lightning-induced dissociation of methane and subsequently upwelled from depth - perhaps embedded within and on the surface of spectrally bright condensates such as ammonium hydrosulfide or ammonia - may be a dominant optical material within the dark thunderstorm-related clouds of Saturn. ?? 2009 Elsevier Ltd. All rights reserved.

Recent Findings Related to Giant Cloud Condensation Nuclei in the Marine Boundary Layer and Impacts on Clouds and Precipitation

NASA Astrophysics Data System (ADS)

Sorooshian, Armin; Dadashazar, Hossein; Wang, Zhen; Crosbie, Ewan; Brunke, Michael; Zeng, Xubin; Jonsson, Haflidi; Woods, Roy; Flagan, Richard; Seinfeld, John

2017-04-01

This presentation reports on findings from multiple airborne field campaigns off the California coast to understand the sources, nature, and impacts of giant cloud condensation nuclei (GCCN). Aside from sea spray emissions, measurements have revealed that ocean-going ships can be a source of GCCN due to wake and stack emissions off the California coast. Observed particle number concentrations behind 10 ships exceeded those in "control" areas, exhibiting number concentration enhancement ratios (ERs) for minimum threshold diameters of 2, 10, and 20 μm as high as 2.7, 5.5, and 7.5, respectively. The data provide insights into how ER is related to a variety of factors (downwind distance, altitude, ship characteristics such as gross tonnage, length, and beam). The data also provide insight into the extent to which a size distribution parameter and a cloud water chemical measurement can capture the effect of sea salt on marine stratocumulus cloud properties. The two GCCN proxy variables, near-surface particle number concentration for diameter > 5 µm and cloud water chloride concentration, are significantly correlated with each other, and both exhibit expected relationships with other parameters that typically coincide with sea salt emissions. Factors influencing the relationship between these two GCCN proxy measurements will be discussed. When comparing twelve pairs of high and low chloride cloud cases (at fixed liquid water path and cloud drop number concentration), the average drop spectra for high chloride cases exhibit enhanced drop number at diameters exceeding 20 µm, especially above 30 µm. In addition, high chloride cases coincide with enhanced mean columnar R and negative values of precipitation susceptibility. The difference in drop effective radius (re) between high and low chloride conditions decreases with height in cloud, suggesting that some GCCN-produced rain drops precipitate before reaching cloud tops. The sign of cloud responses (i.e., re, R) to perturbations in giant sea salt particle concentration, as evaluated from MERRA-2 reanalysis data, is consistent with the aircraft data.

In situ measurements of ship tracks

NASA Technical Reports Server (NTRS)

Radke, Lawrence F.; Lyons, Jamie H.; Hobbs, Peter V.; Coakley, James E.

1990-01-01

It has long been known that cloud droplet concentrations are strongly influenced by cloud condensation nuclei (CCN) and that anthropogenic sources of pollution can affect CCN concentrations. More recently it has been suggested that CCN may play an important role in climate through their effect on cloud albedo. A interesting example of the effect of anthropogenic CCN on cloud albedo is the so-called 'ship track' phenomenon. Ship tracks were first observed in satellite imagery when the ship's emissions were evidently needed for the formation of a visible cloud. However, they appear more frequently in satellite imagery as modifications to existing stratus and stratocumulus clouds. The tracks are seen most clearly in satellite imagery by comparing the radiance at 3.7 microns with that at 0.63 and 11 microns. To account for the observed change in radiance, droplet concentrations must be high, and the mean size of the droplets small, in ship tracks. Researchers describe what they believe to be the first in situ measurements in what appears to have been a ship track.

Why do general circulation models overestimate the aerosol cloud lifetime effect? A case study comparing CAM5 and a CRM

DOE PAGES

Zhou, Cheng; Penner, Joyce E.

2017-01-02

Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water path (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 27 May 2011 at the southern Great Plains (SGP) measurement site established by the Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) program using a single-column version of a global climate model (Community Atmosphere Model or CAM) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP inmore » CAM is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near the cloud top, resulting in an overall decrease in LWP. Lastly, our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.« less

Why do general circulation models overestimate the aerosol cloud lifetime effect? A case study comparing CAM5 and a CRM

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zhou, Cheng; Penner, Joyce E.

Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water path (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 27 May 2011 at the southern Great Plains (SGP) measurement site established by the Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) program using a single-column version of a global climate model (Community Atmosphere Model or CAM) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP inmore » CAM is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near the cloud top, resulting in an overall decrease in LWP. Lastly, our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.« less

Studies of Dark Spots and Their Companion Clouds on the Ice Giant Planets

NASA Astrophysics Data System (ADS)

Bhure, Sakhee; Sankar, Ramanakumar; Hadland, Nathan; Palotai, Csaba J.; Le Beau, Raymond P.; Koutas, Nikko

2017-10-01

Observations of ice giant planets in our Solar System have shown several large-scale dark spots with varying lifespans. Some of these features were directly observed, others were diagnosed from their orographic companion clouds. Historically, numerical simulations have been able to model certain characteristics of these storms such as the shape variability of the Neptune Great Dark Spot (GDS-89) (Deng and Le Beau, 2006), but have not been able to match observed drift rates and lifespans using the standard zonal wind profiles (Hammel et al. 2009). Common amongst these studies has been the lack of condensable species in the atmosphere and an explicit treatment of cloud microphysics. Yet, observations show that dark spots can affect neighboring cloud features, such as in the case of bright companion clouds or the “Berg” on Uranus. An analysis of the cloud structure is therefore required to gain a better understanding of the underlying atmospheric physics and dynamics of these vortices.For our simulations, we use the Explicit Planetary Isentropic Coordinate (EPIC) general circulation model (Dowling et al. 1998, 2006) and adapt its jovian cloud microphysics module which successfully reproduced the cloud structure of jovian storms, such as the Great Red Spot and the Oval BA (Palotai and Dowling 2008, Palotai et al. 2014). EPIC was recently updated to account for the condensation of methane and hydrogen sulfide (Palotai et al. 2016), which allows us to account for both the high-altitude methane ice-cloud and the deep atmosphere hydrogen sulfide ice-cloud layers.In this work, we simulate large-scale vortices on Uranus and Neptune with varying cloud microphysical parameters such as the deep abundance and the ambient supersaturation. We examine the effect of cloud formation on their lifespan and drift rates to better understand the underlying processes which drive these storms.

Understanding aerosol-cloud interactions in the development of orographic cumulus congestus during IPHEx

NASA Astrophysics Data System (ADS)

Barros, A. P.; Duan, Y.

2017-12-01

A new cloud parcel model (CPM) including activation, condensation, collision-coalescence, and lateral entrainment processes is presented here to investigate aerosol-cloud interactions (ACI) in cumulus development prior to rainfall onset. The CPM was employed along with ground based radar and surface aerosol measurements to predict the vertical structure of cloud formation at early stages and evaluated against airborne observations of cloud microphysics and thermodynamic conditions during the Integrated Precipitation and Hydrology Experiment (IPHEx) over the Southern Appalachian Mountains. Further, the CPM was applied to explore the space of ACI physical parameters controlling cumulus congestus growth not available from measurements, and to examine how variations in aerosol properties and microphysical processes influence the evolution and thermodynamic state of clouds over complex terrain via sensitivity analysis. Modeling results indicate that simulated spectra with a low value of condensation coefficient (0.01) are in good agreement with IPHEx aircraft observations around the same altitude. This is in contrast with high values reported in previous studies assuming adiabatic conditions. Entrainment is shown to govern the vertical development of clouds and the change of droplet numbers with height, and the sensitivity analysis suggests that there is a trade-off between entrainment strength and condensation process. Simulated CDNC also exhibits high sensitivity to variations in initial aerosol concentration at cloud base, but weak sensitivity to aerosol hygroscopicity. Exploratory multiple-parcel simulations capture realistic time-scales of vertical development of cumulus congestus (deeper clouds and faster droplet growth). These findings provide new insights into determinant factors of mid-day cumulus congestus formation that can explain a large fraction of warm season rainfall in mountainous regions.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Penner, Joyce E.; Zhou, Cheng

Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water path (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 05/27/2011 at the Southern Great Plains (SGP) measurement site established by Department of Energy's Atmospheric Radiation Measurement (ARM) Program using a single column version of a global climate model (Community Atmosphere Model or CAM) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP in CAMmore » is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near cloud top, resulting in an overall decrease in LWP. Our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.« less

Modeling studying on ice formation by bacteria in warm-based convective cloud

NASA Astrophysics Data System (ADS)

Sun, J.

2005-12-01

Bacteria have been recognized as cloud condensation nuclei (CCN), and certain bacteria, commonly found in plants, have exhibited capacity to act as ice nuclei (IN) at temperatures as warm as -2 °C. These ice nucleating bacteria are readily disseminated into the atmosphere and have been observed in clouds at altitudes of several kilometres. It is noteworthy that over 20 years ago, one assumed the possibility of bacterial transport and their importance into cloud formation process, rain and precipitation, as well as causing disease in plants and animal kingdom. We used a 1-D cumulus cloud model with the CCOPE 19th July 1981 case and the observed field profile of bacterial concentration, to simulate the significance of bacteria as IN through condensation freezing mechanism. In this paper, we will present our results on the role of bacteria as active ice nuclei in the developing stage of cumulus clouds, and their potential significance in atmospheric sciences.

Clouds over Tharsis

NASA Technical Reports Server (NTRS)

1998-01-01

Color composite of condensate clouds over Tharsis made from red and blue images with a synthesized green channel. Mars Orbiter Camera wide angle frames from Orbit 48.

Figure caption from Science Magazine

The clouds of Venus. II - An investigation of the influence of coagulation on the observed droplet size distribution

NASA Technical Reports Server (NTRS)

Rossow, W. B.

1977-01-01

An approximate numerical technique is used to investigate the influence of coagulation, sedimentation and turbulent motions on the observed droplet size distribution in the upper layers of the Venus clouds. If the cloud mass mixing ratio is less than 0.000001 at 250 K or the eddy diffusivity throughout the cloud is greater than 1,000,000 sq cm per sec, then coagulation is unimportant. In this case, the observed droplet size distribution is the initial size distribution produced by the condensation of the droplets. It is found that all cloud models with droplet formation near the cloud top (e.g., a photochemical model) must produce the observed droplet size distribution by condensation without subsequent modification by coagulation. However, neither meteoritic or surface dust can supply sufficient nucleating particles to account for the observed droplet number density. If the cloud droplets are formed near the cloud bottom, the observed droplet size distribution can be produced solely by the interaction of coagulation and dynamics; all information about the initial size distribution is lost. If droplet formation occurs near the cloud bottom, the lower atmosphere of Venus is oxidizing rather than reducing.

Aerosol-cloud interactions in mixed-phase convective clouds - Part 1: Aerosol perturbations

NASA Astrophysics Data System (ADS)

Miltenberger, Annette K.; Field, Paul R.; Hill, Adrian A.; Rosenberg, Phil; Shipway, Ben J.; Wilkinson, Jonathan M.; Scovell, Robert; Blyth, Alan M.

2018-03-01

Changes induced by perturbed aerosol conditions in moderately deep mixed-phase convective clouds (cloud top height ˜ 5 km) developing along sea-breeze convergence lines are investigated with high-resolution numerical model simulations. The simulations utilise the newly developed Cloud-AeroSol Interacting Microphysics (CASIM) module for the Unified Model (UM), which allows for the representation of the two-way interaction between cloud and aerosol fields. Simulations are evaluated against observations collected during the COnvective Precipitation Experiment (COPE) field campaign over the southwestern peninsula of the UK in 2013. The simulations compare favourably with observed thermodynamic profiles, cloud base cloud droplet number concentrations (CDNC), cloud depth, and radar reflectivity statistics. Including the modification of aerosol fields by cloud microphysical processes improves the correspondence with observed CDNC values and spatial variability, but reduces the agreement with observations for average cloud size and cloud top height. Accumulated precipitation is suppressed for higher-aerosol conditions before clouds become organised along the sea-breeze convergence lines. Changes in precipitation are smaller in simulations with aerosol processing. The precipitation suppression is due to less efficient precipitation production by warm-phase microphysics, consistent with parcel model predictions. In contrast, after convective cells organise along the sea-breeze convergence zone, accumulated precipitation increases with aerosol concentrations. Condensate production increases with the aerosol concentrations due to higher vertical velocities in the convective cores and higher cloud top heights. However, for the highest-aerosol scenarios, no further increase in the condensate production occurs, as clouds grow into an upper-level stable layer. In these cases, the reduced precipitation efficiency (PE) dominates the precipitation response and no further precipitation enhancement occurs. Previous studies of deep convective clouds have related larger vertical velocities under high-aerosol conditions to enhanced latent heating from freezing. In the presented simulations changes in latent heating above the 0°C are negligible, but latent heating from condensation increases with aerosol concentrations. It is hypothesised that this increase is related to changes in the cloud field structure reducing the mixing of environmental air into the convective core. The precipitation response of the deeper mixed-phase clouds along well-established convergence lines can be the opposite of predictions from parcel models. This occurs when clouds interact with a pre-existing thermodynamic environment and cloud field structural changes occur that are not captured by simple parcel model approaches.

Xeromorphic traits help to maintain photosynthesis in the perhumid climate of a Taiwanese cloud forest.

PubMed

Pariyar, Shyam; Chang, Shih-Chieh; Zinsmeister, Daniel; Zhou, Haiyang; Grantz, David A; Hunsche, Mauricio; Burkhardt, Juergen

2017-07-01

Previous flux measurements in the perhumid cloud forest of northeastern Taiwan have shown efficient photosynthesis of the endemic tree species Chamaecyparis obtusa var. formosana even under foggy conditions in which leaf surface moisture would be expected. We hypothesized this to be the result of 'xeromorphic' traits of the Chamaecyparis leaves (hydrophobicity, stomatal crypts, stomatal clustering), which could prevent coverage of stomata by precipitation, fog, and condensation, thereby maintaining CO 2 uptake. Here we studied the amount, distribution, and composition of moisture accumulated on Chamaecyparis leaf surfaces in situ in the cloud forest. We studied the effect of surface tension on gas penetration to stomata using optical O 2 microelectrodes in the laboratory. We captured the dynamics of condensation to the leaf surfaces with an environmental scanning electron microscope (ESEM). In spite of substantial surface hydrophobicity, the mean water film thickness on branchlets under foggy conditions was 80 µm (upper surface) and 40 µm (lower surface). This amount of water could cover stomata and prevent CO 2 uptake. This is avoided by the clustered arrangement of stomata within narrow clefts and the presence of Florin rings. These features keep stomatal pores free from water due to surface tension and provide efficient separation of plant and atmosphere in this perhumid environment. Air pollutants, particularly hygroscopic aerosol, may disturb this functionality by enhancing condensation and reducing the surface tension of leaf surface water.

Distinct Impacts of Aerosols on an Evolving Continental Cloud Complex during the RACORO Field Campaign

DOE PAGES

Lin, Yun; Wang, Yuan; Pan, Bowen; ...

2016-08-26

In this study, a continental cloud complex, consisting of shallow cumuli, a deep convective cloud (DCC), and stratus, is simulated by a cloud-resolving Weather Research and Forecasting Model to investigate the aerosol microphysical effect (AME) and aerosol radiative effect (ARE) on the various cloud regimes and their transitions during the Department of Energy Routine Atmospheric Radiation Measurement Aerial Facility Clouds with Low Optical Water Depths Optical Radiative Observations (RACORO) campaign. Under an elevated aerosol loading with AME only, a reduced cloudiness for the shallow cumuli and stratus resulted from more droplet evaporation competing with suppressed precipitation, but an enhanced cloudinessmore » for the DCC is attributed to more condensation. With the inclusion of ARE, the shallow cumuli are suppressed owing to the thermodynamic effects of light-absorbing aerosols. The responses of DCC and stratus to aerosols are monotonic with AME only but nonmonotonic with both AME and ARE. The DCC is invigorated because of favorable convection and moisture conditions at night induced by daytime ARE, via the so-called aerosol-enhanced conditional instability mechanism. Finally, the results reveal that the overall aerosol effects on the cloud complex are distinct from the individual cloud types, highlighting that the aerosol–cloud interactions for diverse cloud regimes and their transitions need to be evaluated to assess the regional and global climatic impacts.« less

Aerosol-Cloud Interactions and Cloud Microphysical Properties in the Asir Region of Saudi Arabia

NASA Astrophysics Data System (ADS)

Kucera, P. A.; Axisa, D.; Burger, R. P.; Li, R.; Collins, D. R.; Freney, E. J.; Buseck, P. R.

2009-12-01

In recent advertent and inadvertent weather modification studies, a considerable effort has been made to understand the impact of varying aerosol properties and concentration on cloud properties. Significant uncertainties exist with aerosol-cloud interactions for which complex microphysical processes link the aerosol and cloud properties. Under almost all environmental conditions, increased aerosol concentrations within polluted air masses will enhance cloud droplet concentration relative to that in unperturbed regions. The interaction between dust particles and clouds are significant, yet the conditions in which dust particles become cloud condensation nuclei (CCN) are uncertain. In order to quantify this aerosol effect on clouds and precipitation, a field campaign was launched in the Asir region, located adjacent to the Red Sea in the southwest region of Saudi Arabia. Ground measurements of aerosol size distributions, hygroscopic growth factors, CCN concentrations as well as aircraft measurements of cloud hydrometeor size distributions were observed in the Asir region in August 2009. The presentation will include a summary of the analysis and results with a focus on aerosol-cloud interactions and cloud microphysical properties observed during the convective season in the Asir region.

Use of In Situ Cloud Condensation Nuclei, Extinction, and Aerosol Size Distribution Measurements to Test a Method for Retrieving Cloud Condensation Nuclei Profiles From Surface Measurements

NASA Technical Reports Server (NTRS)

Ghan, Stephen J.; Rissman, Tracey A.; Ellman, Robert; Ferrare, Richard A.; Turner, David; Flynn, Connor; Wang, Jian; Ogren, John; Hudson, James; Jonsson, Haflidi H.;

A Novel Effect of Scattered-Light Interference in Misted Mirrors

ERIC Educational Resources Information Center

Bridge, N. James

2005-01-01

Interference rings can be observed in mirrors clouded by condensation, even in diffuse lighting. The effect depends on individual droplets acting as point sources by refracting light into the mirror, so producing coherent wave-trains which are reflected and then scattered again by diffraction round the same source droplet. The secondary wave-train…

A numerical study of the effect of different aerosol types on East Asian summer clouds and precipitation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jiang, Yiquan; Liu, Xiaohong; Yang, Xiuqun

2013-05-01

The impact of anthropogenic aerosol on the East Asian summer monsoon (EASM) is investigated with NCAR CAM5, a state-of-the-art climate model with aerosol’s direct and indirect effects. Results indicate that anthropogenic aerosol tends to cause a weakened EASM with a southward shift of precipitation in East Asia mostly by its radiative effect. Anthropogenic aerosol induced surface cooling stabilizes the boundary layer, suppresses the convection and latent heat release in northern China, and reduces the tropospheric temperature over land and land-sea thermal contrast, thus leading to a weakened EASM. Meanwhile, acting as cloud condensation nuclei (CCN), anthropogenic aerosol can significantly increasemore » the cloud droplet number concentration but decrease the cloud droplet effective radius over Indochina and Indian Peninsulas as well as over southwestern and northern China, inhibiting the precipitation in these regions. Thus, anthropogenic aerosol tends to reduce Southeast and South Asian summer monsoon precipitation by its indirect effect.« less

Effects of Wildfire Pollution on the Microphysical and Electrical Properties of Pyrocumulus

NASA Astrophysics Data System (ADS)

Duff, R.; Grant, L. D.; van den Heever, S. C.

2014-12-01

Pyrocumulus clouds form over wildfires when hot, smoke-filled air rises, cools and condenses. These clouds have higher cloud condensation nuclei (CCN) concentrations, which affect their microphysical and electrical properties. It is important to better understand pyrocumulus cloud microphysical characteristics and lightning formation, which have implications for the prediction of wildfire growth as well as the radiative and chemical characteristics of the upper troposphere. A recent observational study documented an electrified pyrocumulus over the May 2012 Hewlett Gulch fire located to the west of Fort Collins, Colorado. This cloud produced approximately 20 intracloud lightning flashes, and its electrical activity differed from surrounding convection that was not directly impacted by the fire and associated smoke. The goal of this research is to investigate aerosol-induced cloud-scale microphysical differences between clean clouds and polluted pyrocumulus to better characterize the mechanisms that cause pyrocumulus electrification. In order to address this goal, idealized cloud-resolving model simulations were performed using the Regional Atmospheric Modeling System (RAMS). The model environment was initialized with an average of the 12Z 16 May and 00Z 17 May 2012 observed Denver soundings to represent the conditions when the Hewlett Gulch pyrocumulus occurred. Five simulations were performed using surface aerosol concentrations from 100 to 5000 #/mg. The results demonstrate that in moderately polluted pyrocumulus, rain processes are suppressed while graupel production increases. Extremely polluted pyrocumulus, however, experience a complete shut-down of graupel production, which favors the production of large amounts of liquid water and smaller ice species such as ice crystals and snowflakes. The processes responsible for these microphysical changes, as well as inferred pyrocumulus electrification mechanisms, will be compared with those discussed in previous observational studies of this case.

Simulation of seasonal cloud forcing anomalies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Randall, D.A.

1990-08-01

One useful way to classify clouds is according to the processes that generate them. There are three main cloud-formation agencies: deep convection; surface evaporation; large-scale lifting in the absence of conditional instability. Although traditionally clouds have been viewed as influencing the atmospheric general circulation primarily through the release of latent heat, the atmospheric science literature contains abundant evidence that, in reality, clouds influence the general circulation through four more or less equally important effects: interactions with the solar and terrestrial radiation fields; condensation and evaporation; precipitation; small-scale circulations within the atmosphere. The most advanced of the current generation of GCMsmore » include parameterizations of all four effects. Until recently there has been lingering skepticism, in the general circulation modeling community, that the radiative effects of clouds significantly influence the atmospheric general circulation. GCMs have provided the proof that the radiative effects of clouds are important for the general circulation of the atmosphere. An important concept in analysis of the effects of clouds on climate is the cloud radiative forcing (CRF), which is defined as the difference between the radiative flux which actually occurs in the presence of clouds, and that which would occur if the clouds were removed but the atmospheric state were otherwise unchanged. We also use the term CRF to denote warming or cooling tendencies due to cloud-radiation interactions. Cloud feedback is the change in CRF that accompanies a climate change. The present study concentrates on the planetary CRF and its response to external forcing, i.e. seasonal change.« less

Approach for measuring the chemistry of individual particles in the size range critical for cloud formation.

PubMed

Zauscher, Melanie D; Moore, Meagan J K; Lewis, Gregory S; Hering, Susanne V; Prather, Kimberly A

2011-03-15

Aerosol particles, especially those ranging from 50 to 200 nm, strongly impact climate by serving as nuclei upon which water condenses and cloud droplets form. However, the small number of analytical methods capable of measuring the composition of particles in this size range, particularly at the individual particle level, has limited our knowledge of cloud condensation nuclei (CCN) composition and hence our understanding of aerosols effect on climate. To obtain more insight into particles in this size range, we developed a method which couples a growth tube (GT) to an ultrafine aerosol time-of-flight mass spectrometer (UF-ATOFMS), a combination that allows in situ measurements of the composition of individual particles as small as 38 nm. The growth tube uses water to grow particles to larger sizes so they can be optically detected by the UF-ATOFMS, extending the size range to below 100 nm with no discernible changes in particle composition. To gain further insight into the temporal variability of aerosol chemistry and sources, the GT-UF-ATOFMS was used for online continuous measurements over a period of 3 days.

Substantial convection and precipitation enhancements by ultrafine aerosol particles

NASA Astrophysics Data System (ADS)

Fan, Jiwen; Rosenfeld, Daniel; Zhang, Yuwei; Giangrande, Scott E.; Li, Zhanqing; Machado, Luiz A. T.; Martin, Scot T.; Yang, Yan; Wang, Jian; Artaxo, Paulo; Barbosa, Henrique M. J.; Braga, Ramon C.; Comstock, Jennifer M.; Feng, Zhe; Gao, Wenhua; Gomes, Helber B.; Mei, Fan; Pöhlker, Christopher; Pöhlker, Mira L.; Pöschl, Ulrich; de Souza, Rodrigo A. F.

2018-01-01

Ultrafine aerosol particles (smaller than 50 nanometers in diameter) have been thought to be too small to affect cloud formation. Fan et al. show that this is not the case. They studied the effect of urban pollution transported into the otherwise nearly pristine atmosphere of the Amazon. Condensational growth of water droplets around the tiny particles releases latent heat, thereby intensifying atmospheric convection. Thus, anthropogenic ultrafine aerosol particles may exert a more important influence on cloud formation processes than previously believed.

Clouds over Tharsis

NASA Image and Video Library

1998-03-13

Color composite of condensate clouds over Tharsis made from red and blue images with a synthesized green channel. Mars Orbiter Camera wide angle frames from Orbit 48. http://photojournal.jpl.nasa.gov/catalog/PIA00812

Organic cloud condensation nuclei: the effect of phase, surface tension, trace soluble species, and oxidative processing on particle activation.

NASA Astrophysics Data System (ADS)

Broekhuizen, K. E.; Thornberry, T.; Abbatt, J. P.

2003-12-01

The ability of organic aerosols to act as cloud condensation nuclei (CCN) will be discussed. A variety of laboratory experiments will be presented which address several key questions concerning organic particle activation. Does the particle phase impact activation? How does surface tension play a role and can a trace amount of a surface active species impact activation? Does a trace amount of a highly soluble species impact the activation of organic particles of moderate to low solubility? Can the activation properties of organic aerosols be enhanced through oxidative processing? To systematically address these issues, the CCN activity of various diacids such as oxalic, malonic, succinic, adipic and azelaic acid have been studied, as well as the addition of trace amounts of nonanoic acid and ammonium sulfate to examine the roles of surface active and soluble species, respectively. The first examination of the role of oxidative processing on CCN activity has involved investigating the effect of ozone oxidation on the activity of oleic acid particles.

New particle formation and growth in biomass burning plumes: An important source of cloud condensation nuclei

NASA Astrophysics Data System (ADS)

Hennigan, Christopher J.; Westervelt, Daniel M.; Riipinen, Ilona; Engelhart, Gabriella J.; Lee, Taehyoung; Collett, Jeffrey L., Jr.; Pandis, Spyros N.; Adams, Peter J.; Robinson, Allen L.

2012-05-01

Experiments were performed in an environmental chamber to characterize the effects of photo-chemical aging on biomass burning emissions. Photo-oxidation of dilute exhaust from combustion of 12 different North American fuels induced significant new particle formation that increased the particle number concentration by a factor of four (median value). The production of secondary organic aerosol caused these new particles to grow rapidly, significantly enhancing cloud condensation nuclei (CCN) concentrations. Using inputs derived from these new data, global model simulations predict that nucleation in photo-chemically aging fire plumes produces dramatically higher CCN concentrations over widespread areas of the southern hemisphere during the dry, burning season (Sept.-Oct.), improving model predictions of surface CCN concentrations. The annual indirect forcing from CCN resulting from nucleation and growth in biomass burning plumes is predicted to be -0.2 W m-2, demonstrating that this effect has a significant impact on climate that has not been previously considered.

Direct Numerical Simulation of Turbulent Condensation in Clouds

NASA Technical Reports Server (NTRS)

Shariff, K.; Paoli, R.

2004-01-01

In this brief, we investigate the turbulent condensation of a population of droplets by means of a direct numerical simulation. To that end, a coupled Navier-Stokes/Lagrangian solver is used where each particle is tracked and its growth by water vapor condensation is monitored exactly. The main goals of the study are to find out whether turbulence broadens the droplet size distribution, as observed in in situ measurements. The second issue is to understand if and for how long a correlation between the droplet radius and the local supersaturation exists for the purpose of modeling sub-grid scale microphysics in cloud-resolving codes. This brief is organized as follows. In Section 2 the governing equations are presented, including the droplet condensation model. The implementation of the forcing procedure is described in Section 3. The simulation results are presented in Section 4 together with a sketch of a simple stochastic model for turbulent condensation. Conclusions and the main outcomes of the study are given in Section 5.

Cloud Properties Derived from Surface-Based Near-Infrared Spectral Transmission

NASA Technical Reports Server (NTRS)

Pilewskie, Peter; Twomey, S.; Gore, Warren J. Y. (Technical Monitor)

1996-01-01

Surface based near-infrared cloud spectral transmission measurements from a recent precipitation/cloud physics field study are used to determine cloud physical properties and relate them to other remote sensing and in situ measurements. Asymptotic formulae provide an effective means of closely approximating the qualitative and quantitative behavior of transmission computed by more laborious detailed methods. Relationships derived from asymptotic formulae are applied to measured transmission spectra to test objectively the internal consistency of data sets acquired during the field program and they confirmed the quality of the measurements. These relationships appear to be very useful in themselves, not merely as a quality control measure, but also a potentially valuable remote-sensing technique in its own right. Additional benefits from this analysis have been the separation of condensed water (cloud) transmission and water vapor transmission and the development of a method to derive cloud liquid water content.

Inhomogeneities in frontal cirrus clouds

NASA Astrophysics Data System (ADS)

Neis, Patrick; Krämer, Martina; Hoor, Peter; Reutter, Philipp; Spichtinger, Peter

2013-04-01

Frontal cirrus clouds have a scientifically proven effect on the Earth's radiation budget and thereby an influence on the weather and climate change in regional scale. The formation processes and structures of frontal cirrus clouds are still not fully understood. For a close investigation of typical frontal cirrus clouds, we use in situ measurements from the CIRRUS-III campaign over Germany and Northern Europe in November 2006. Besides water vapour, cloud ice water content, ice particle size distributions, condensation nuclei, and reactive nitrogen were measured during 6 flights. In this work the data of the 24th November flight is used to detect and to analyze warm frontal cirrus clouds in the mid latitudes on small temporal and spatial scale. Further, these results are compared with large-scale meteorological analyses from ECMWF and satellite data. Combining these data, the formation and evolution of inhomogeneities in the cirrus cloud structure are investigated. One important result is a qualitative agreement between the occurrence of cirrus clouds and the 'sharpness' of the Tropopause Inversion Layer (TIL).

Organic condensation: A vital link connecting aerosol formation to climate forcing (Invited)

NASA Astrophysics Data System (ADS)

Riipinen, I.; Pierce, J. R.; Yli-Juuti, T.; Nieminen, T.; Häkkinen, S.; Ehn, M.; Junninen, H.; Lehtipalo, K.; Petdjd, T. T.; Slowik, J. G.; Chang, R. Y.; Shantz, N. C.; Abbatt, J.; Leaitch, W. R.; Kerminen, V.; Worsnop, D. R.; Pandis, S. N.; Donahue, N. M.; Kulmala, M. T.

2010-12-01

Aerosol-cloud interactions represent the largest uncertainty in calculations of Earth’s radiative forcing. Number concentrations of atmospheric aerosol particles are in the core of this uncertainty, as they govern the numbers of cloud condensation nuclei (CCN) and influence the albedo and lifetime of clouds. Aerosols also impair air quality through their adverse effects on atmospheric visibility and human health. The ultrafine fraction (<100 nm) of atmospheric aerosol particles often dominates the total aerosol numbers, and nucleation of atmospheric vapours is one of the most important sources of these particles. To have climatic relevance, however, the freshly-nucleated particles need to grow in size, and consequently their climatic importance remains to be quantified (see Fig. 1). We combine observations from two continental sites (Egbert, Canada and Hyytiälä, Finland) to show that condensation of organic vapours is a crucial factor governing the lifetimes and climatic importance of the smallest atmospheric particles. We demonstrate that state-of-the-science organic gas-particle partitioning models fail to reproduce the observations; we propose a new modelling approach that is consistent with the measurements. Finally, we demonstrate the large sensitivity of climatic forcing of atmospheric aerosols to these interactions between organic vapours and the smallest atmospheric nanoparticles - highlighting the need for representing this process in global climate models. Figure 1. Organic emissions and the dynamic processes governing the climatic importance of ultrafine aerosol. Condensable vapours are produced upon oxidation of volatile organic compounds (VOCs) and can 1) nucleate to form new small particles; 2) grow freshly formed particles to larger sizes and increase their probability to serve as CCN; 3) condense on the background aerosol (> 100 nm) and enhance the loss of ultrafine particles. Primary organic aerosol (POA) contributes to the large end of the aerosol size distribution, enhancing the scavenging of the ultrafine particles.

Mars atmospheric CO2 condensation above the north and south poles as revealed by radio occultation, climate sounder, and laser ranging observations

NASA Astrophysics Data System (ADS)

Hu, Renyu; Cahoy, Kerri; Zuber, Maria T.

2012-07-01

We study the condensation of CO2 in Mars' atmosphere using temperature profiles retrieved from radio occultation measurements from Mars Global Surveyor (MGS) as well as the climate sounding instrument onboard the Mars Reconnaissance Orbiter (MRO), and detection of reflective clouds by the MGS Mars Orbiter Laser Altimeter (MOLA). We find 11 events in 1999 where MGS temperature profiles indicate CO2 condensation and MOLA simultaneously detects reflective clouds. We thus provide causal evidence that MOLA non-ground returns are associated with CO2 condensation, which strongly indicates their nature being CO2 clouds. The MGS and MRO temperature profiles together reveal the seasonal expansion and shrinking of the area and the vertical extent of atmospheric saturation. The occurrence rate of atmospheric saturation is maximized at high latitudes in the middle of winter. The atmospheric saturation in the northern polar region exhibits more intense seasonal variation than in the southern polar region. In particular, a shrinking of saturation area and thickness from LS ˜ 270° to ˜300° in 2007 is found; this is probably related to a planet-encircling dust storm. Furthermore, we integrate the condensation area and the condensation occurrence rate to estimate cumulative masses of CO2 condensates deposited onto the northern and southern seasonal polar caps. The precipitation flux is approximated by the particle settling flux which is estimated using the impulse responses of MOLA filter channels. With our approach, the total atmospheric condensation mass can be estimated from these observational data sets with average particle size as the only free parameter. By comparison with the seasonal polar cap masses inferred from the time-varying gravity of Mars, our estimates indicate that the average condensate particle radius is 8-22 μm in the northern hemisphere and 4-13 μm in the southern hemisphere. Our multi-instrument data analysis provides new constraints on modeling the global climate of Mars.

The Surface Energy Budget and Precipitation Efficiency for Convective Systems During TOGA, COARE, GATE, SCSMEX and ARM: Cloud-Resolving Model Simulations

NASA Technical Reports Server (NTRS)

Tao, W.-K.; Shie, C.-L.; Johnson, D; Simpson, J.; Starr, David OC. (Technical Monitor)

2002-01-01

A two-dimensional version of the Goddard Cumulus Ensemble (GCE) Model is used to simulate convective systems that developed in various geographic locations. Observed large-scale advective tendencies for potential temperature, water vapor mixing ratio, and horizontal momentum derived from field campaigns are used as the main forcing. By examining the surface energy budgets, the model results show that the two largest terms are net condensation (heating/drying) and imposed large-scale forcing (cooling/moistening) for tropical oceanic cases. These two terms arc opposite in sign, however. The contributions by net radiation and latent heat flux to the net condensation vary in these tropical cases, however. For cloud systems that developed over the South China Sea and eastern Atlantic, net radiation (cooling) accounts for about 20% or more of the net condensation. However, short-wave heating and long-wave cooling are in balance with each other for cloud systems over the West Pacific region such that the net radiation is very small. This is due to the thick anvil clouds simulated in the cloud systems over the Pacific region. Large-scale cooling exceeds large-scale moistening in the Pacific and Atlantic cases. For cloud systems over the South China Sea, however, there is more large-scale moistening than cooling even though the cloud systems developed in a very moist environment. though For three cloud systems that developed over a mid-latitude continent, the net radiation and sensible and latent heat fluxes play a much more important role. This means the accurate measurement of surface fluxes and radiation is crucial for simulating these mid-latitude cases.

Long-term observation of aerosol cloud relationships in the Mid-Atlantic region

NASA Astrophysics Data System (ADS)

Li, S.; Joseph, E.; Min, Q.; Yin, B.

2013-12-01

Long-term ground-based observations of aerosol and cloud properties derived from measurements of Multifilter Rotating Shadow Band Radiometer and microwave radiometer at an atmospheric measurement field station in the Baltimore-Washington corridor operated by Howard University are used to examine the temporal variation of aerosol and cloud properties and moreover aerosol indirect effect on clouds. Through statistical analysis of five years (from 2006 to 2010) of these observations, the proportion of polluted cases is found larger in 2006 and 2007 and the proportion of optically thick clouds cases is also larger in 2006 and 2007 than that in 2008, 2009 and 2010. Both the mean aerosol optical depth (AOD) and cloud optical depth (COD) are observed decreasing from 2006 to 2010 but there is no obvious trend observed on cloud liquid water path (LWP). Because of the limit of AOD retrievals under cloudy conditions surface measurements of fine particle particulate matter 2.5 (PM2.5) were used for assessing aerosol indirect effect. A positive relationship between LWP and cloud droplets effective radius (Re) and a negative relationship between PM2.5 and Re are observed based on a stringent case selection method which is used to reduce the uncertainties from retrieval and meteorological impacts. The total 5 years summer time observations are segregated according to the value of PM2.5. Examination of distributions of COD, cloud condensation nuclei (CCN), cloud droplets effective radius and LWP under polluted and pristine conditions further confirm that the high aerosol loading decreases cloud droplets effective radius and increases cloud optical depth.

The Role of Long-Lived Greenhouse Gases as Principal LW Control Knob that Governs the Global Surface Temperature for Past and Future Climate Change

NASA Technical Reports Server (NTRS)

Lacis, Andrew A.; Hansen, James E.; Russell, Gary L.; Oinas, Valdar; Jonas, Jeffrey

2013-01-01

The climate system of the Earth is endowed with a moderately strong greenhouse effect that is characterized by non-condensing greenhouse gases (GHGs) that provide the core radiative forcing. Of these, the most important is atmospheric CO2. There is a strong feedback contribution to the greenhouse effect by water vapor and clouds that is unique in the solar system, exceeding the core radiative forcing due to the non-condensing GHGs by a factor of three. The significance of the non-condensing GHGs is that once they have been injected into the atmosphere, they remain there virtually indefinitely because they do not condense and precipitate from the atmosphere, their chemical removal time ranging from decades to millennia. Water vapor and clouds have only a short lifespan, with their distribution determined by the locally prevailing meteorological conditions, subject to Clausius-Clapeyron constraint. Although solar irradiance is the ultimate energy source that powers the terrestrial greenhouse effect, there has been no discernible long-term trend in solar irradiance since precise monitoring began in the late 1970s. This leaves atmospheric CO2 as the effective control knob driving the current global warming trend. Over geological time scales, volcanoes are the principal source of atmospheric CO2, and the weathering of rocks is the principal sink, with the biosphere participating as both a source and a sink. The problem at hand is that human industrial activity is causing atmospheric CO2, to increase by 2 ppm per year, whereas the interglacial rate has been 0.005 ppm per year. This is a geologically unprecedented rate to turn the CO2 climate control knob. This is causing the global warming that threatens the global environment.

New particle formation leads to cloud dimming

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sullivan, Ryan C.; Crippa, Paola; Matsui, Hitoshi

New particle formation (NPF), nucleation of condensable vapors to the solid or liquid phase, is a significant source of atmospheric aerosol particle number concentrations. With sufficient growth, these nucleated particles may be a significant source of cloud condensation nuclei (CCN), thus altering cloud albedo, structure, and lifetimes, and insolation reaching the Earth's surface. Herein we present one of the first numerical experiments to quantify the impact of NPF on cloud radiative properties that is conducted at a convection permitting resolution and that explicitly simulates cloud droplet number concentrations. Consistent with observations, these simulations suggest that in spring over the Midwesternmore » U.S.A., NPF occurs frequently and on regional scales. However, the simulations suggest that NPF is not associated with enhancement of regional cloud albedos as would be expected from an increase of CCN. These simulations indicate that NPF reduces ambient sulfuric acid concentrations sufficiently to inhibit growth of preexisting particles to CCN sizes. This reduction in CCN-sized particles reduces cloud albedo, resulting in a domain average positive top of atmosphere cloud radiative forcing of 10 W m-2 and up to ~ 50 W m-2 in individual grid cells relative to a simulation in which NPF is excluded.« less

Properties of Arctic Aerosol Particles and Residuals of Warm Clouds: Cloud Activation Efficiency and the Aerosol Indirect Effect

NASA Astrophysics Data System (ADS)

Zelenyuk, A.; Imre, D. G.; Leaitch, R.; Ovchinnikov, M.; Liu, P.; Macdonald, A.; Strapp, W.; Ghan, S. J.; Earle, M. E.

2012-12-01

Single particle mass spectrometer, SPLAT II, was used to characterize the size, composition, number concentration, density, and shape of individual Arctic spring aerosol. Background particles, particles above and below the cloud, cloud droplet residuals, and interstitial particles were characterized with goal to identify the properties that separate cloud condensation nuclei (CCN) from background aerosol particles. The analysis offers a comparison between warm clouds formed on clean and polluted days, with clean days having maximum particle concentrations (Na) lower than ~250 cm-3, as compared with polluted days, in which maximum concentration was tenfold higher. On clean days, particles were composed of organics, organics mixed with sulfates, biomass burning (BB), sea salt (SS), and few soot and dust particles. On polluted days, BB, organics associated with BB, and their mixtures with sulfate dominated particle compositions. Based on the measured compositions and size distributions of cloud droplet residuals, background aerosols, and interstitial particles, we conclude that these three particle types had virtually the same compositions, which means that cloud activation probabilities were surprisingly nearly composition independent. Moreover, these conclusions hold in cases in which less than 20% or more than 90% of background particles got activated. We concluded that for the warm clouds interrogated in this study particle size played a more important factor on aerosol CCN activity. Comparative analysis of all studied clouds reveals that aerosol activation efficiency strongly depends on the aerosol concentrations, such that at Na <200 cm-3, nearly all particles activate, and at higher concentrations the activation efficiency is lower. For example, when Na was greater than 1500 cm-3, less than ~30% of particles activated. The data suggest that as the number of nucleated droplets increases, condensation on existing droplets effectively competes with particle activation, limiting maximum droplet concentrations Nd = 525 ± 50 cm-3, which is lower than the 750 cm-3 limit found by Leaitch et al. (1986) for mid-latitude continental cloud that had generally larger updraft speeds than the clouds interrogated in Arctic. These findings are important for the aerosol indirect effect, in which increase in aerosol particle number concentrations is expected to result in increase in Nd and decrease in droplet size, leading to increased cloud albedo and potentially lifetimes. Our conclusions point to limited susceptibility to changes in ambient aerosol concentrations, providing simple explanation for the finding of weaker than expected indirect effect. In summary, the data presented here show that Nd increases as the cloud base particle number concentration increases; however, they also show a limit on Nd that is in the range of 500-600 cm-3.

On the probability distribution function of the mass surface density of molecular clouds. I

NASA Astrophysics Data System (ADS)

Fischera, Jörg

2014-05-01

The probability distribution function (PDF) of the mass surface density is an essential characteristic of the structure of molecular clouds or the interstellar medium in general. Observations of the PDF of molecular clouds indicate a composition of a broad distribution around the maximum and a decreasing tail at high mass surface densities. The first component is attributed to the random distribution of gas which is modeled using a log-normal function while the second component is attributed to condensed structures modeled using a simple power-law. The aim of this paper is to provide an analytical model of the PDF of condensed structures which can be used by observers to extract information about the condensations. The condensed structures are considered to be either spheres or cylinders with a truncated radial density profile at cloud radius rcl. The assumed profile is of the form ρ(r) = ρc/ (1 + (r/r0)2)n/ 2 for arbitrary power n where ρc and r0 are the central density and the inner radius, respectively. An implicit function is obtained which either truncates (sphere) or has a pole (cylinder) at maximal mass surface density. The PDF of spherical condensations and the asymptotic PDF of cylinders in the limit of infinite overdensity ρc/ρ(rcl) flattens for steeper density profiles and has a power law asymptote at low and high mass surface densities and a well defined maximum. The power index of the asymptote Σ- γ of the logarithmic PDF (ΣP(Σ)) in the limit of high mass surface densities is given by γ = (n + 1)/(n - 1) - 1 (spheres) or by γ = n/ (n - 1) - 1 (cylinders in the limit of infinite overdensity). Appendices are available in electronic form at http://www.aanda.org

Influence of Microphysical Variability on Stochastic Condensation in Turbulent Clouds

NASA Astrophysics Data System (ADS)

Desai, N.; Chandrakar, K. K.; Chang, K.; Glienke, S.; Cantrell, W. H.; Fugal, J. P.; Shaw, R. A.

2017-12-01

We investigate the influence of variability in droplet number concentration and radius on the evolution of cloud droplet size distributions. Measurements are made on the centimeter scale using digitial inline holography, both in a controlled laboratory setting and in the field using HOLODEC measurements from CSET. We created steady state cloud conditions in the laboratory Pi Chamber, in which a turbulent cloud can be sustained for long periods of time. Using holographic imaging, we directly observe the variations in local number concentration and droplet size distribution and, thereby, the integral radius. We interpret the measurements in the context of stochastic condensation theory to determine how fluctuations in integral radius contribute to droplet growth. We find that the variability in integral radius is primarily driven by variations in the droplet number concentration and not the droplet radius. This variability does not contribute significantly to the mean droplet growth rate, but contributes significantly to the rate of increase of the size distribution width. We compare these results with in-situ measurements and find evidence for microphysical signatures of stochastic condensation. The results suggest that supersaturation fluctuations lead to broader size distributions and allow droplets to reach the collision-coalescence stage.

Sensitivity of a Cumulus Parameterization Scheme to Precipitation Production Representation and Its Impact on a Heavy Rain Event over Korea

DOE Office of Scientific and Technical Information (OSTI.GOV)

Han, Ji-Young; Hong, Song-You; Sunny Lim, Kyo-Sun

The sensitivity of a cumulus parameterization scheme (CPS) to a representation of precipitation production is examined. To do this, the parameter that determines the fraction of cloud condensate converted to precipitation in the simplified Arakawa–Schubert (SAS) convection scheme is modified following the results from a cloud-resolving simulation. While the original conversion parameter is assumed to be constant, the revised parameter includes a temperature dependency above the freezing level, whichleadstolessproductionoffrozenprecipitating condensate with height. The revised CPS has been evaluated for a heavy rainfall event over Korea as well as medium-range forecasts using the Global/Regional Integrated Model system (GRIMs). The inefficient conversionmore » of cloud condensate to convective precipitation at colder temperatures generally leads to a decrease in pre-cipitation, especially in the category of heavy rainfall. The resultant increase of detrained moisture induces moistening and cooling at the top of clouds. A statistical evaluation of the medium-range forecasts with the revised precipitation conversion parameter shows an overall improvement of the forecast skill in precipitation and large-scale fields, indicating importance of more realistic representation of microphysical processes in CPSs.« less

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

NASA Technical Reports Server (NTRS)

Tao, Wei-Kuo; Khain, A.; Simpson, S.; Johnson, D.; Li, X.; Remer, L.

2003-01-01

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e.,pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bin model explicitly calculates and allows for the examination of both the mass and number concentration of species in each size categor, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fewer droplets, larger sized develop due to the greater condensational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Can Condensing Organic Aerosols Lead to Less Cloud Particles?

NASA Astrophysics Data System (ADS)

Gao, C. Y.; Tsigaridis, K.; Bauer, S.

2017-12-01

We examined the impact of condensing organic aerosols on activated cloud number concentration in a new aerosol microphysics box model, MATRIX-VBS. The model includes the volatility-basis set (VBS) framework in an aerosol microphysical scheme MATRIX (Multiconfiguration Aerosol TRacker of mIXing state) that resolves aerosol mass and number concentrations and aerosol mixing state. Preliminary results show that by including the condensation of organic aerosols, the new model (MATRIX-VBS) has less activated particles compared to the original model (MATRIX), which treats organic aerosols as non-volatile. Parameters such as aerosol chemical composition, mass and number concentrations, and particle sizes which affect activated cloud number concentration are thoroughly evaluated via a suite of Monte-Carlo simulations. The Monte-Carlo simulations also provide information on which climate-relevant parameters play a critical role in the aerosol evolution in the atmosphere. This study also helps simplifying the newly developed box model which will soon be implemented in the global model GISS ModelE as a module.

Particles from a Diesel ship engine: Mixing state on the nano scale and cloud condensation abilities

NASA Astrophysics Data System (ADS)

Lieke, K. I.; Rosenørn, T.; Fuglsang, K.; Frederiksen, T.; Butcher, A. C.; King, S. M.; Bilde, M.

2012-04-01

Transport by ship plays an important role in global logistics. Current international policy initiatives by the International Maritime Organization (IMO) are taken to reduce emissions from ship propulsion systems (NO and SO, primarily). However, particulate emissions (e.g. soot) from ships are yet not regulated by legislations. To date, there is still a lack of knowledge regarding the global and local effects of the particulate matter emitted from ships at sea. Particles may influence the climate through their direct effects (scattering and absorption of long and shortwave radiation) and indirectly through formation of clouds. Many studies have been carried out estimating the mass and particle number from ship emissions (e.g. Petzold et al. 2008), many of them in test rig studies (e.g. Kasper et al. 2007). It is shown that particulate emissions vary with engine load and chemical composition of fuels. Only a few studies have been carried out to characterize the chemical composition and cloud-nucleating ability of the particulate matter (e.g. Corbett et al. 1997). In most cases, the cloud-nucleating ability of emission particles is estimated from number size distribution. We applied measurements to characterize particulate emissions from a MAN B&W Low Speed engine on test bed. A unique data set was obtained through the use of a scanning mobility particle sizing system (SMPS), combined with a cloud condensation nucleus (CCN) counter and a thermodenuder - all behind a dilution system. In addition, impactor samples were taken on nickel grids with carbon foil for use in an electron microscope (EM) to characterize the mineral phase and mixing state of the particles. The engine was operated at a series of different load conditions and an exhaust gas recirculation (EGR) system was applied. Measurements were carried out before and after the EGR system respectively. Our observations show significant changes in number size distribution and CCN activity with varying conditions. Results of transmission electron microscopy revealed salt condensates of nanometer size attached to soot particles. High resolution structural analysis of single particles shows that three different phases (graphitic soot, crystalline salt and amorphous condensed organic matter) may be present in the same particle volume. A closure between CCN activation curves, EM samples, and SMPS size distribution will be presented and used to identify climate active parts in single particles. ACKNOWLEDGEMENTS We thank the Danish Agency for Science, Technology and Innovation for support through the NaKIM project (www.nakim.dk).

A Linearized Prognostic Cloud Scheme in NASAs Goddard Earth Observing System Data Assimilation Tools

NASA Technical Reports Server (NTRS)

Holdaway, Daniel; Errico, Ronald M.; Gelaro, Ronald; Kim, Jong G.; Mahajan, Rahul

2015-01-01

A linearized prognostic cloud scheme has been developed to accompany the linearized convection scheme recently implemented in NASA's Goddard Earth Observing System data assimilation tools. The linearization, developed from the nonlinear cloud scheme, treats cloud variables prognostically so they are subject to linearized advection, diffusion, generation, and evaporation. Four linearized cloud variables are modeled, the ice and water phases of clouds generated by large-scale condensation and, separately, by detraining convection. For each species the scheme models their sources, sublimation, evaporation, and autoconversion. Large-scale, anvil and convective species of precipitation are modeled and evaporated. The cloud scheme exhibits linearity and realistic perturbation growth, except around the generation of clouds through large-scale condensation. Discontinuities and steep gradients are widely used here and severe problems occur in the calculation of cloud fraction. For data assimilation applications this poor behavior is controlled by replacing this part of the scheme with a perturbation model. For observation impacts, where efficiency is less of a concern, a filtering is developed that examines the Jacobian. The replacement scheme is only invoked if Jacobian elements or eigenvalues violate a series of tuned constants. The linearized prognostic cloud scheme is tested by comparing the linear and nonlinear perturbation trajectories for 6-, 12-, and 24-h forecast times. The tangent linear model performs well and perturbations of clouds are well captured for the lead times of interest.

Water ice clouds on Mars: a study of partial cloudiness with a global climate model and MARCI data

NASA Astrophysics Data System (ADS)

Pottier, Alizée; Montmessin, Franck; Forget, François; Wolff, Mike; Navarro, Thomas; Millour, Ehouarn; Madeleine, Jean-Baptiste; Spiga, Aymeric; Bertrand, Tanguy

2015-04-01

There is a large reservoir of water ice on Mars in the polar caps, that sublimates in summer and releases water vapor. Water is then advected in the atmospheric circulation that evolves seasonally. This vapor forms clouds, frost, and can also be adsorbed in the soil. In a global study of the water cycle, water ice clouds play a key part in the martian climate. There is a need to understand better their distribution and radiative effect. The tool used in this study is the global climate model (GCM) of the Laboratoire de Météorologie Dynamique. It is made up of a core that computes fluid dynamics, and a physical part that gathers a number of parametrised processes. It includes tracers and the condensation and sublimation of water in the atmosphere and on the ground, allowing a study of the complete water cycle. To improve the representation of water ice clouds in the model, a new parametrisation of partial cloudiness has been implemented and will be presented. Indeed, model cells are hundreds of kilometers wide, and it is quite unrealistic to suppose that cloud coverage is always uniform in them. Furthermore, the model was quite unstable since the implementation of the radiative effect of clouds, and partial cloudiness had the effect of reducing this instability. In practice, a subgrid temperature distribution is supposed, and the temperature computed in the model is interpreted as its mean. The subgrid scale temperature distribution is simple, and its width is a free parameter. Using this distribution, the fraction of the grid cells under the water vapor condensation temperature is interpreted as the fraction of the cell in which clouds form (or cloud fraction). From these fractions at each height a total partial cloudiness (the clouds as seen from the orbit) is deduced. The radiative transfer is computed twice, for the clear area and for the cloudy one. Observing the water cycle with this new parametrisation, some differences are seen with standard runs. These changes mainly affect the aphelion cloud belt and the polar hoods. Partial cloudiness is compared to higher resolution (one per one degree) runs in which cloudiness diagnostics are done. MARCI data of cloud opacity is also used to verify the predicted water ice cloud distribution and patchiness. The aim is to understand the causes of patchiness and to validate the choice of a subgrid scale temperature distribution. There are seasonal variations, recurring patterns near major topographical features.

Cloud Condensation Nuclei in Cumulus Humilis - Selected Case Study During the CHAPS Campaign

NASA Astrophysics Data System (ADS)

Yu, X.; Berg, L. K.; Berkowitz, C. M.; Alexander, M. L.; Lee, Y.; Laskin, A.; Ogren, J. A.; Andrews, B.

2009-12-01

The Cumulus Humilis Aerosol Processing Study (CHAPS) provided a unique opportunity to study aerosol and cloud processing. Clouds play an active role in the processing and cycling of atmospheric constituents. Gases and particles can partition to cloud droplets by absorption and condensation as well as activation and pact scavenging. The Department of Energy (DOE) G-1 aircraft was used as one of the main platforms in CHAPS. Flight tracks were designed and implemented to characterize freshly emitted aerosols on cloud top and cloud base as well as with cloud, i.e., cumulus humilis (or fair-weather cumulus), in the vicinity of Oklahoma City. Measurements of interstitial aerosols and residuals of activated condensation cloud nuclei were conducted simultaneously. The interstitial aerosols were determined downstream of an isokinetic inlet; and the activated particles downstream of a counter-flow virtual impactor (CVI). The sampling line to the Aerodyne Aerosol Mass Spectrometer was switched between the isokinetic inlet and the CVI to allow characterization of interstitial particles out of clouds in contrast to particles activated in clouds. Trace gases including ozone, carbon monoxide, sulfur dioxide, and a series of volatile organic compounds (VOCs) were also measured as were key meteorological state parameters including liquid water content, cloud drop size, and dew point temperature were measured. This work will focus on studying CCN properties in cumulus humilis. Several approaches will be taken. The first is single particle analysis of particles collected by the Time-Resolved Aerosol Sampler (TRAC) by SEM/TEM coupled with EDX. We will specifically look into differences in particle properties such as chemical composition and morphology between activated and interstitial ones. The second analysis will link in situ measurements with the snap shots observations by TRAC. For instance, by looking into the characteristic m/z obtained by AMS vs. CO or isoprene, one can gain more insight into the role of primary and secondary organic aerosols in CCNs and background aerosols. Combined with observations of cloud properties, an improved picture of CCN activation in cumulus humilis can be made.

Direct Observations of Clouds on Brown Dwarfs: A Spitzer Study of Extreme Cases

NASA Astrophysics Data System (ADS)

Burgasser, Adam; Cruz, Kelle; Cushing, Michael; Kirkpatrick, J. Davy; Looper, Dagny; Lowrance, Patrick; Marley, Mark; Saumon, Didier

2008-03-01

Clouds play a fundamental role in the emergent spectral energy distributions and observed variability of very low mass stars and brown dwarfs, yet hey have only been studied indirectly thus far. Recent indications of a broad silicate grain absorption feature in the 8-11 micron spectra of mid-type L dwarfs, and evidence that the strength of this absorption varies according to broad-band near-infrared color, may finally allow the first direct studies of clouds and condensate grain properties in brown dwarf atmospheres. We propose to observe a sample of 18 ``extreme'' L dwarfs - objects with unusually blue and red near-infrared colors - with IRAC and IRS to study the 8-11 micron feature in detail (including grain size distributions and bulk compositions), and to constrain advanced condensate cloud atmosphere models currently in development. Our program provides a unique examination of the general processes of cloud formation by focusing on the relatively warm photospheres of late-type brown dwarfs.

Turbulence and star formation in molecular clouds

NASA Astrophysics Data System (ADS)

Larson, R. B.

1981-03-01

Consideration is given to the turbulence properties of molecular clouds and their implications for star formation. Data for 54 molecular clouds and condensations is presented which reveals cloud velocity dispersion and region size to follow a power-law relation, similar to the Kolmogoroff law for subsonic turbulence. Examination of the dynamics of the molecular clouds for which mass determinations are available reveals essentially all of them to be gravitationally bound, and to approximately satisfy the virial theorem. The observation of moderate scatter in the dispersion-size relation is noted to imply that most regions have not collapsed much since formation, suggesting that processes of turbulent hydrodynamics have played an important role in producing the observed substructures. A lower limit to the size of subcondensations at which their internal motions are no longer supersonic is shown to predict a minimum protostellar mass on the order of a few tenths of a solar mass, while massive protostellar clumps are found to develop complex internal structures, probably leading to the formation of prestellar condensation nuclei. The observed turbulence of molecular clouds is noted to imply lifetimes of less than 10 million years.

Trade-Wind Cloudiness and Climate

NASA Technical Reports Server (NTRS)

Randall, David A.

1997-01-01

Closed Mesoscale Cellular Convection (MCC) consists of mesoscale cloud patches separated by narrow clear regions. Strong radiative cooling occurs at the cloud top. A dry two-dimensional Bousinesq model is used to study the effects of cloud-top cooling on convection. Wide updrafts and narrow downdrafts are used to indicate the asymmetric circulations associated with the mesoscale cloud patches. Based on the numerical results, a conceptual model was constructed to suggest a mechanism for the formation of closed MCC over cool ocean surfaces. A new method to estimate the radioative and evaporative cooling in the entrainment layer of a stratocumulus-topped boundary layer has been developed. The method was applied to a set of Large-Eddy Simulation (LES) results and to a set of tethered-balloon data obtained during FIRE. We developed a statocumulus-capped marine mixed layer model which includes a parameterization of drizzle based on the use of a predicted Cloud Condensation Nuclei (CCN) number concentration. We have developed, implemented, and tested a very elaborate new stratiform cloudiness parameterization for use in GCMs. Finally, we have developed a new, mechanistic parameterization of the effects of cloud-top cooling on the entrainment rate.

Microphysical response of cloud droplets in a fluctuating updraft. Ph.D. Thesis

NASA Technical Reports Server (NTRS)

Harding, D. D.

1977-01-01

The effect of a fluctuating updraft upon a distribution of cloud droplets is examined. Computations are performed for fourteen vertical velocity patterns; each allows a closed parcel of cloud air to undergo downward as well as upward motion. Droplet solution and curvature effects are included. The classical equations for the growth rate of an individual droplet by vapor condensation relies on simplifying assumptions. Those assumptions are isolated and examined. A unique approach is presented in which all energy sources and sinks of a droplet may be considered and is termed the explicit model. It is speculated that the explicit model may enhance the growth of large droplets at greater heights. Such a model is beneficial to the studies of pollution scavenging and acid rain.

Hemispheric aerosol vertical profiles: anthropogenic impacts on optical depth and cloud nuclei.

PubMed

Clarke, Antony; Kapustin, Vladimir

2010-09-17

Understanding the effect of anthropogenic combustion upon aerosol optical depth (AOD), clouds, and their radiative forcing requires regionally representative aerosol profiles. In this work, we examine more than 1000 vertical profiles from 11 major airborne campaigns in the Pacific hemisphere and confirm that regional enhancements in aerosol light scattering, mass, and number are associated with carbon monoxide from combustion and can exceed values in unperturbed regions by more than one order of magnitude. Related regional increases in a proxy for cloud condensation nuclei (CCN) and AOD imply that direct and indirect aerosol radiative effects are coupled issues linked globally to aged combustion. These profiles constrain the influence of combustion on regional AOD and CCN suitable for challenging climate model performance and informing satellite retrievals.

Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon.

PubMed

Pöschl, U; Martin, S T; Sinha, B; Chen, Q; Gunthe, S S; Huffman, J A; Borrmann, S; Farmer, D K; Garland, R M; Helas, G; Jimenez, J L; King, S M; Manzi, A; Mikhailov, E; Pauliquevis, T; Petters, M D; Prenni, A J; Roldin, P; Rose, D; Schneider, J; Su, H; Zorn, S R; Artaxo, P; Andreae, M O

2010-09-17

The Amazon is one of the few continental regions where atmospheric aerosol particles and their effects on climate are not dominated by anthropogenic sources. During the wet season, the ambient conditions approach those of the pristine pre-industrial era. We show that the fine submicrometer particles accounting for most cloud condensation nuclei are predominantly composed of secondary organic material formed by oxidation of gaseous biogenic precursors. Supermicrometer particles, which are relevant as ice nuclei, consist mostly of primary biological material directly released from rainforest biota. The Amazon Basin appears to be a biogeochemical reactor, in which the biosphere and atmospheric photochemistry produce nuclei for clouds and precipitation sustaining the hydrological cycle. The prevailing regime of aerosol-cloud interactions in this natural environment is distinctly different from polluted regions.

Rainforest Aerosols as Biogenic Nuclei of Clouds and Precipitation in the Amazon

NASA Astrophysics Data System (ADS)

Pöschl, U.; Martin, S. T.; Sinha, B.; Chen, Q.; Gunthe, S. S.; Huffman, J. A.; Borrmann, S.; Farmer, D. K.; Garland, R. M.; Helas, G.; Jimenez, J. L.; King, S. M.; Manzi, A.; Mikhailov, E.; Pauliquevis, T.; Petters, M. D.; Prenni, A. J.; Roldin, P.; Rose, D.; Schneider, J.; Su, H.; Zorn, S. R.; Artaxo, P.; Andreae, M. O.

2010-09-01

The Amazon is one of the few continental regions where atmospheric aerosol particles and their effects on climate are not dominated by anthropogenic sources. During the wet season, the ambient conditions approach those of the pristine pre-industrial era. We show that the fine submicrometer particles accounting for most cloud condensation nuclei are predominantly composed of secondary organic material formed by oxidation of gaseous biogenic precursors. Supermicrometer particles, which are relevant as ice nuclei, consist mostly of primary biological material directly released from rainforest biota. The Amazon Basin appears to be a biogeochemical reactor, in which the biosphere and atmospheric photochemistry produce nuclei for clouds and precipitation sustaining the hydrological cycle. The prevailing regime of aerosol-cloud interactions in this natural environment is distinctly different from polluted regions.

Mars Atmospheric CO2 Condensation Above the North and South Poles as Revealed by Radio Occultation, Climate Sounder, and Laser Ranging Observations

NASA Technical Reports Server (NTRS)

Hu, Renyu; Cahoy, Kerri; Zuber, Maria T.

2012-01-01

We study the condensation of CO2 in Mars atmosphere using temperature profilesretrieved from radio occultation measurements from Mars Global Surveyor (MGS) as wellas the climate sounding instrument onboard the Mars Reconnaissance Orbiter (MRO),and detection of reflective clouds by the MGS Mars Orbiter Laser Altimeter (MOLA). Wefind 11 events in 1999 where MGS temperature profiles indicate CO2 condensation andMOLA simultaneously detects reflective clouds. We thus provide causal evidence thatMOLA non-ground returns are associated with CO2 condensation, which strongly indicatestheir nature being CO2 clouds. The MGS and MRO temperature profiles together revealthe seasonal expansion and shrinking of the area and the vertical extent of atmosphericsaturation. The occurrence rate of atmospheric saturation is maximized at high latitudes inthe middle of winter. The atmospheric saturation in the northern polar region exhibits moreintense seasonal variation than in the southern polar region. In particular, a shrinking ofsaturation area and thickness from LS 270 to 300 in 2007 is found; this is probablyrelated to a planet-encircling dust storm. Furthermore, we integrate the condensation areaand the condensation occurrence rate to estimate cumulative masses of CO2 condensatesdeposited onto the northern and southern seasonal polar caps. The precipitation flux isapproximated by the particle settling flux which is estimated using the impulse responses ofMOLA filter channels. With our approach, the total atmospheric condensation mass canbe estimated from these observational data sets with average particle size as the onlyfree parameter. By comparison with the seasonal polar cap masses inferred from thetime-varying gravity of Mars, our estimates indicate that the average condensate particleradius is 822 mm in the northern hemisphere and 413 mm in the southern hemisphere.Our multi-instrument data analysis provides new constraints on modeling the global climateof Mars.

Aerosol Microphysical and Radiative Effects on Continental Cloud Ensembles

DOE PAGES

Wang, Yuan; Vogel, Jonathan M.; Lin, Yun; ...

2018-01-10

Aerosol-cloud-radiation interactions represent one of the largest uncertainties in the current climate assessment. Much of the complexity arises from the non-monotonic responses of clouds, precipitation and radiative fluxes to aerosol perturbations under various meteorological conditions. Here, an aerosol-aware Weather Research and Forecasting (WRF) model is used to investigate the microphysical and radiative effects of aerosols in three weather systems during the March 2000 Cloud Intensive Observational Period campaign at the Southern Great Plains site of the US Atmospheric Radiation Measurement Program. Three cloud ensembles with different meteorological conditions are simulated, including a low-pressure deep convective cloud system, a series ofmore » lessprecipitating stratus and shallow cumulus, and a cold frontal passage. The WRF simulations are evaluated by the available observations of cloud fraction, liquid water path, precipitation, and surface temperature. The microphysical properties of cloud hydrometeors, such as their mass and number concentrations, generally show monotonic trends as a function of cloud condensation nuclei concentrations. Aerosol radiative effects do not interfere the trends of cloud microphysics, except for the stratus and shallow cumulus cases where aerosol semi-direct effects are identified. The precipitation changes by aerosols vary with the cloud types and their evolving stages, with more prominent aerosol invigoration effect and associated enhanced precipitation from the convective sources. Furthermore, the simulated aerosol direct effect suppresses precipitation in all three cases but does not overturn the direction of precipitation changes by the aerosol indirect effect. Cloud fraction exhibits much smaller sensitivity (typically less than 2%) to aerosol perturbations than the cloud microphysics, and the responses vary with aerosol concentrations and cloud regimes. The surface shortwave radiation shows a monotonic decrease by increasing aerosols, while the magnitude of the decrease depends on the cloud type. Surface temperature changes closely follow the modulation of the surface radiation fluxes.« less

Aerosol Microphysical and Radiative Effects on Continental Cloud Ensembles

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, Yuan; Vogel, Jonathan M.; Lin, Yun

Aerosol-cloud-radiation interactions represent one of the largest uncertainties in the current climate assessment. Much of the complexity arises from the non-monotonic responses of clouds, precipitation and radiative fluxes to aerosol perturbations under various meteorological conditions. Here, an aerosol-aware Weather Research and Forecasting (WRF) model is used to investigate the microphysical and radiative effects of aerosols in three weather systems during the March 2000 Cloud Intensive Observational Period campaign at the Southern Great Plains site of the US Atmospheric Radiation Measurement Program. Three cloud ensembles with different meteorological conditions are simulated, including a low-pressure deep convective cloud system, a series ofmore » lessprecipitating stratus and shallow cumulus, and a cold frontal passage. The WRF simulations are evaluated by the available observations of cloud fraction, liquid water path, precipitation, and surface temperature. The microphysical properties of cloud hydrometeors, such as their mass and number concentrations, generally show monotonic trends as a function of cloud condensation nuclei concentrations. Aerosol radiative effects do not interfere the trends of cloud microphysics, except for the stratus and shallow cumulus cases where aerosol semi-direct effects are identified. The precipitation changes by aerosols vary with the cloud types and their evolving stages, with more prominent aerosol invigoration effect and associated enhanced precipitation from the convective sources. Furthermore, the simulated aerosol direct effect suppresses precipitation in all three cases but does not overturn the direction of precipitation changes by the aerosol indirect effect. Cloud fraction exhibits much smaller sensitivity (typically less than 2%) to aerosol perturbations than the cloud microphysics, and the responses vary with aerosol concentrations and cloud regimes. The surface shortwave radiation shows a monotonic decrease by increasing aerosols, while the magnitude of the decrease depends on the cloud type. Surface temperature changes closely follow the modulation of the surface radiation fluxes.« less

Condensed Acids In Antartic Stratospheric Clouds

NASA Technical Reports Server (NTRS)

Pueschel, R. F.; Snetsinger, K. G.; Toon, O. B.; Ferry, G. V.; Starr, W. L.; Oberbeck, V. R.; Chan, K. R.; Goodman, J. K.; Livingston, J. M.; Verma, S.;

Participation in the Mars Data Analysis Program: Analysis of cloud forms in Viking and Mariner 9 images

NASA Technical Reports Server (NTRS)

Gierasch, P.; Kahn, R. A.

1985-01-01

The first systematic account of the climate of Mars, based upon observations was produced. Cloud data were used to determine spatially and temporally varying near-surface wind direction, relative wind speed, static stability, and humidity conditions on a global scale. Existing models of meteorological processes were critically reexamined in light of the data, and more stringent constraints were set on global processes. Several discoveries were made, including the large extent and seasonal variability of the Mars equatorial Hadley cell, the failure of high latitude winds to reverse direction in early northern spring, the change in meridional wind component in southern midautum, and the almost constant cloud cover in the northern hemisphere, during spring and summer primarily by condensate clouds and in fall and winter by condensates and dust. The implications of these observations are discussed.

CHEMISTRY OF SILICATE ATMOSPHERES OF EVAPORATING SUPER-EARTHS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schaefer, Laura; Fegley, Bruce, E-mail: laura_s@levee.wustl.ed, E-mail: bfegley@levee.wustl.ed

2009-10-01

We model the formation of silicate atmospheres on hot volatile-free super-Earths. Our calculations assume that all volatile elements such as H, C, N, S, and Cl have been lost from the planet. We find that the atmospheres are composed primarily of Na, O{sub 2}, O, and SiO gas, in order of decreasing abundance. The atmospheric composition may be altered by fractional vaporization, cloud condensation, photoionization, and reaction with any residual volatile elements remaining in the atmosphere. Cloud condensation reduces the abundance of all elements in the atmosphere except Na and K. We speculate that large Na and K clouds suchmore » as those observed around Mercury and Io may surround hot super-Earths. These clouds would occult much larger fractions of the parent star than a closely bound atmosphere, and may be observable through currently available methods.« less

Galileo's Earth-Moon portrait

NASA Astrophysics Data System (ADS)

Simarski, Lynn Teo

Research reported at an AGU session on Galileo's Earth/Moon flyby refined the spacecraft's distinctive portrait of the Earth-Moon system. The Galileo team presented dramatic new views of the Earth and Moon taken last December. Andrew P. Ingersoll showed a color movie of the rotating Earth, made through spectral filters with which Galileo viewed the Earth almost continuously for 25 hours.Galileo also made finely tuned observations of vegetation and clouds, using three very closely spaced spectral wavelengths in the near-infrared, explained W. Reid Thompson. In the resulting images, Argentinian grassland and Brazilian rain forest are clearly distinguished, demonstrating the applicability of this technique for routine monitoring of deforestation, shifts in vegetation due to climate, and other phenomena. Thompson suggested that this capability could be used on the Earth Observing System. One of the spectral bands may also have potential for monitoring cloud condensation, as it appears to differentiate actively condensing, vapor-heavy clouds from higher and drier clouds.

Clouds in the Martian Atmosphere

NASA Astrophysics Data System (ADS)

Määttänen, Anni; Montmessin, Franck

2018-01-01

Although resembling an extremely dry desert, planet Mars hosts clouds in its atmosphere. Every day somewhere on the planet a part of the tiny amount of water vapor held by the atmosphere can condense as ice crystals to form cirrus-type clouds. The existence of water ice clouds has been known for a long time, and they have been studied for decades, leading to the establishment of a well-known climatology and understanding of their formation and properties. Despite their thinness, they have a clear impact on the atmospheric temperatures, thus affecting the Martian climate. Another, more exotic type of clouds forms as well on Mars. The atmospheric temperatures can plunge to such frigid values that the major gaseous component of the atmosphere, CO2, condenses as ice crystals. These clouds form in the cold polar night where they also contribute to the formation of the CO2 ice polar cap, and also in the mesosphere at very high altitudes, near the edge of space, analogously to the noctilucent clouds on Earth. The mesospheric clouds are a fairly recent discovery and have put our understanding of the Martian atmosphere to a test. On Mars, cloud crystals form on ice nuclei, mostly provided by the omnipresent dust. Thus, the clouds link the three major climatic cycles: those of the two major volatiles, H2O and CO2; and that of dust, which is a major climatic agent itself.

Solid-State Photochemistry as a Formation Mechanism for Titan's Stratospheric C4N2 Ice Clouds

NASA Technical Reports Server (NTRS)

Anderson, C. M.; Samuelson, R. E.; Yung, Y. L.; McLain, J. L.

2016-01-01

We propose that C4N2 ice clouds observed in Titan's springtime polar stratosphere arise due to solid-state photochemistry occurring within extant ice cloud particles of HCN-HC3N mixtures. This formation process resembles the halogen-induced ice particle surface chemistry that leads to condensed nitric acid trihydrate (NAT) particles and ozone depletion in Earth's polar stratosphere. As our analysis of the Cassini Composite Infrared Spectrometer 478 per centimeter ice emission feature demonstrates, this solid-state photochemistry mechanism eliminates the need for the relatively high C4N2 saturation vapor pressures required (even though they are not observed) when the ice is produced through the usual procedure of direct condensation from the vapor.

Rain scavenging of solid rocket exhaust clouds

NASA Technical Reports Server (NTRS)

Dingle, A. N.

1978-01-01

An explicit model for cloud microphysics was developed for application to the problem of co-condensation/vaporization of HCl and H2O in the presence of Al2O3 particulate nuclei. Validity of the explicit model relative to the implicit model, which has been customarily applied to atmospheric cloud studies, was demonstrated by parallel computations of H2O condensation upon (NH4)2 SO4 nuclei. A mesoscale predictive model designed to account for the impact of wet processes on atmospheric dynamics is also under development. Input data specifying the equilibrium state of HC1 and H2O vapors in contact with aqueous HC1 solutions were found to be limited, particularly in respect to temperature range.

Global aerosol effects on convective clouds

NASA Astrophysics Data System (ADS)

Wagner, Till; Stier, Philip

2013-04-01

Atmospheric aerosols affect cloud properties, and thereby the radiation balance of the planet and the water cycle. The influence of aerosols on clouds is dominated by increase of cloud droplet and ice crystal numbers (CDNC/ICNC) due to enhanced aerosols acting as cloud condensation and ice nuclei. In deep convective clouds this increase in CDNC/ICNC is hypothesised to increase precipitation because of cloud invigoration through enhanced freezing and associated increased latent heat release caused by delayed warm rain formation. Satellite studies robustly show an increase of cloud top height (CTH) and precipitation with increasing aerosol optical depth (AOD, as proxy for aerosol amount). To represent aerosol effects and study their influence on convective clouds in the global climate aerosol model ECHAM-HAM, we substitute the standard convection parameterisation, which uses one mean convective cloud for each grid column, with the convective cloud field model (CCFM), which simulates a spectrum of convective clouds, each with distinct values of radius, mixing ratios, vertical velocity, height and en/detrainment. Aerosol activation and droplet nucleation in convective updrafts at cloud base is the primary driver for microphysical aerosol effects. To produce realistic estimates for vertical velocity at cloud base we use an entraining dry parcel sub cloud model which is triggered by perturbations of sensible and latent heat at the surface. Aerosol activation at cloud base is modelled with a mechanistic, Köhler theory based, scheme, which couples the aerosols to the convective microphysics. Comparison of relationships between CTH and AOD, and precipitation and AOD produced by this novel model and satellite based estimates show general agreement. Through model experiments and analysis of the model cloud processes we are able to investigate the main drivers for the relationship between CTH / precipitation and AOD.

Analysis of African Biomass Burning Over the South East Atlantic and its Interaction with Stratocumulus Clouds during ORACLES 2016/17

NASA Astrophysics Data System (ADS)

Freitag, S.; Howell, S. G.; Dobracki, A. N.; Smirnow, N.; Winchester, C.; Sedlacek, A. J., III; Podolske, J. R.; Noone, D.; McFarquhar, G. M.; Poellot, M.; Delene, D. J.

2017-12-01

During NASA ORACLES 2016/17 airborne missions, biomass burning (BB) advected from the African continent out over the South East Atlantic was intensively studied to better understand the role of BB aerosol in the regional radiation budget but also to discern its effect from natural aerosol on underlying Stratocumulus (Sc) clouds in the marine boundary layer (MBL). Because of its particle size and vast quantities BB aerosol once entrained into the MBL are highly effective as cloud condensation nuclei (CCN) impacting cloud microphysical properties and as such the Sc deck's radiative budget. This work identifies characteristic in-plume size resolved aerosol physiochemistry observed during the campaign with focus on absorbing aerosol measurements retrieved with a Single Particle Soot Photometer (SP2). The results are compared to MBL aerosol obervations and adjacent Sc cloud properties such as the cloud droplet number concentration. Additionally, size resolved aerosol physiochemistry and black carbon concentration were measured in the cloud occasionally using a Counterflow Virtual Impactor (CVI) inlet sampling exclusively cloud droplet residuals. Employing the CVI cloud droplets are inertially separated from the air and dried in-situ en-route to the aerosol instrumentation. This allows us to study natural and combustion-influenced aerosol that were actually activated as CCN in the Sc deck.

Exploring The Relation Between Upper Tropospheric (UT) Clouds and Convection

NASA Astrophysics Data System (ADS)

Stephens, G. L.; Stubenrauch, C.

2017-12-01

The importance of knowing the vertical transports of water vapor and condensate by atmospheric moist convection cannot be overstated. Vertical convective transports have wide-ranging influences on the Earth system, shaping weather, climate, the hydrological cycle and the composition of the atmosphere. These transports also influence the upper tropospheric cloudiness that exerts profound effects on climate. Although there are presently no direct observations to quantify these transports on the large scale, and there are no observations to constrain model assumptions about them, it might be possible to derive useful observations proxies of these transports and their influence. This talk will present results derived from a large community effort that has developed important observations data records that link clouds and convection. Steps to use these observational metrics to examine the relation between convection, UT clouds in both cloud and global scale models are exemplified and important feedbacks between high clouds, radiation and convection will be elucidated.

Marine Aerosols and Clouds.

PubMed

Brooks, Sarah D; Thornton, Daniel C O

2018-01-03

The role of marine bioaerosols in cloud formation and climate is currently so uncertain that even the sign of the climate forcing is unclear. Marine aerosols form through direct emissions and through the conversion of gas-phase emissions to aerosols in the atmosphere. The composition and size of aerosols determine how effective they are in catalyzing the formation of water droplets and ice crystals in clouds by acting as cloud condensation nuclei and ice nucleating particles, respectively. Marine organic aerosols may be sourced both from recent regional phytoplankton blooms that add labile organic matter to the surface ocean and from long-term global processes, such as the upwelling of old refractory dissolved organic matter from the deep ocean. Understanding the formation of marine aerosols and their propensity to catalyze cloud formation processes are challenges that must be addressed given the major uncertainties associated with aerosols in climate models.

Environmental conditions regulate the impact of plants on cloud formation

PubMed Central

Zhao, D. F.; Buchholz, A.; Tillmann, R.; Kleist, E.; Wu, C.; Rubach, F.; Kiendler-Scharr, A.; Rudich, Y.; Wildt, J.; Mentel, Th. F.

2017-01-01

The terrestrial vegetation emits large amounts of volatile organic compounds (VOC) into the atmosphere, which on oxidation produce secondary organic aerosol (SOA). By acting as cloud condensation nuclei (CCN), SOA influences cloud formation and climate. In a warming climate, changes in environmental factors can cause stresses to plants, inducing changes of the emitted VOC. These can modify particle size and composition. Here we report how induced emissions eventually affect CCN activity of SOA, a key parameter in cloud formation. For boreal forest tree species, insect infestation by aphids causes additional VOC emissions which modifies SOA composition thus hygroscopicity and CCN activity. Moderate heat increases the total amount of constitutive VOC, which has a minor effect on hygroscopicity, but affects CCN activity by increasing the particles' size. The coupling of plant stresses, VOC composition and CCN activity points to an important impact of induced plant emissions on cloud formation and climate. PMID:28218253

Environmental conditions regulate the impact of plants on cloud formation.

PubMed

Zhao, D F; Buchholz, A; Tillmann, R; Kleist, E; Wu, C; Rubach, F; Kiendler-Scharr, A; Rudich, Y; Wildt, J; Mentel, Th F

2017-02-20

The terrestrial vegetation emits large amounts of volatile organic compounds (VOC) into the atmosphere, which on oxidation produce secondary organic aerosol (SOA). By acting as cloud condensation nuclei (CCN), SOA influences cloud formation and climate. In a warming climate, changes in environmental factors can cause stresses to plants, inducing changes of the emitted VOC. These can modify particle size and composition. Here we report how induced emissions eventually affect CCN activity of SOA, a key parameter in cloud formation. For boreal forest tree species, insect infestation by aphids causes additional VOC emissions which modifies SOA composition thus hygroscopicity and CCN activity. Moderate heat increases the total amount of constitutive VOC, which has a minor effect on hygroscopicity, but affects CCN activity by increasing the particles' size. The coupling of plant stresses, VOC composition and CCN activity points to an important impact of induced plant emissions on cloud formation and climate.

Study on Cloud Water Resources and Precipitation Efficiency Characteristic over China

NASA Astrophysics Data System (ADS)

Zhou, Y., Sr.; Cai, M., Jr.

2017-12-01

The original concept and quantitative assessment method of cloud water resource and its related physical parameters are proposed based on the atmospheric water circulation and precipitation enhancement. A diagnosis method of the three-dimensional (3-D) cloud and cloud water field are proposed , based on cloud observation and atmospheric reanalysis data. Furthermore, using analysis data and precipitation products, Chinese cloud water resources in 2008-2010 are assessed preliminarily. The results show that: 1. Atmospheric water cycle and water balance plays an important part of the climate system. Water substance includes water vapor and hydrometeors, and the water cycle is the process of phase transition of water substances. Water vapor changes its phase into solid or liquid hydrometeors by lifting and condensation, and after that, the hydrometeors grow lager through cloud physical processes and then precipitate to ground, which is the mainly resource of available fresh water .Therefore, it's far from enough to only focus on the amount of water vapor, more attention should be transfered to the hydrometeors (cloud water resources) which is formed by the process of phase transition including lifting and condensation. The core task of rainfall enhancement is to develop the cloud water resources and raise the precipitation efficiency by proper technological measures. 2. Comparing with the water vapor, the hydrometeor content is much smaller. Besides, the horizontal delivery amount also shows two orders of magnitude lower than water vapor. But the update cycle is faster and the precipitation efficiency is higher. The amount of cloud water resources in the atmosphere is determined by the instantaneous quantity, the advection transport, condensation and precipitation from the water balance.The cloud water resources vary a lot in different regions. In southeast China, hydrometeor has the fastest renewal cycle and the highest precipitation efficiency. The total amount of hydrometeor in the northwest China is relatively small, but it still has some development potential due to the low precipitation efficiency. 3. The accuracy of the assessment results can be improved and the estimation error can be reduced by using higher-resolution reanalysis data or combining of observational diagnosis and numerical model.

The Role of CO2 Clouds on the Stability of the Early Mars Atmosphere Against Collapse

NASA Astrophysics Data System (ADS)

Kahre, Melinda A.; Haberle, Robert; Steakley, Kathryn; Murphy, Jim; Kling, Alexandre

2017-10-01

The early Mars atmosphere was likely significantly more massive than it is today, given the growing body of evidence that liquid water flowed on the surface early in the planet’s history. Although the CO2 inventory was likely larger in the past, there is much we still do not understand about the state of that CO2. As surface pressure increases, the temperature at which CO2 condenses also increases, making it more likely that CO2 ice would form and persist on the surface when the atmospheric mass increases. An atmosphere that is stable against collapse must contain enough energy, distributed globally, to prohibit the formation of permanents CO2 ice reservoirs that lead to collapse. The presence of the “faint young sun” compounds this issue. Previous global climate model (GCM) investigations show that atmospheres within specific ranges of obliquities and atmospheric masses are stable against collapse. We use the NASA Ames Mars GCM to expand on these works by focusing specifically on the role of CO2 clouds in atmospheric stability. Two end member simulations are executed, one that includes CO2 cloud formation and one that does not. The simulation that explicitly includes CO2 clouds is stable, while the simulation without CO2 clouds collapses into permanent surface CO2 reservoirs. In both cases, significant atmospheric condensation is occurring in the atmosphere throughout the year. In the case without CO2 clouds, all atmospheric condensation (even if it occurs at altitude) leads directly to the accumulation of surface ice, whereas in the case with CO2 clouds, there is a finite settling timescale for the cloud particles. Depending on this timescale and the local conditions, the cloud particles could stay aloft or sublimate as they fall toward the surface. Thus, the striking difference between these two cases illustrates the important role of CO2 clouds. We plan to conduct and present further simulations to better understand how atmospheric stability depends on the details of CO2 cloud microphysical processes and assumptions.

A cloud-resolving model study of aerosol-cloud correlation in a pristine maritime environment

NASA Astrophysics Data System (ADS)

Nishant, Nidhi; Sherwood, Steven C.

2017-06-01

In convective clouds, satellite-observed deepening or increased amount of clouds with increasing aerosol concentration has been reported and is sometimes interpreted as aerosol-induced invigoration of the clouds. However, such correlations can be affected by meteorological factors that affect both aerosol and clouds, as well as observational issues. In this study, we examine the behavior in a 660 × 660 km2 region of the South Pacific during June 2007, previously found by Koren et al. (2014) to show strong correlation between cloud fraction, cloud top pressure, and aerosols, using a cloud-resolving model with meteorological boundary conditions specified from a reanalysis. The model assumes constant aerosol loading, yet reproduces vigorous clouds at times of high real-world aerosol concentrations. Days with high- and low-aerosol loading exhibit deep-convective and shallow clouds, respectively, in both observations and the simulation. Synoptic analysis shows that vigorous clouds occur at times of strong surface troughs, which are associated with high winds and advection of boundary layer air from the Southern Ocean where sea-salt aerosol is abundant, thus accounting for the high correlation. Our model results show that aerosol-cloud relationships can be explained by coexisting but independent wind-aerosol and wind-cloud relationships and that no cloud condensation nuclei effect is required.

Global circulation as the main source of cloud activity on Titan

USGS Publications Warehouse

Rodriguez, S.; Le, Mouelic S.; Rannou, P.; Tobie, G.; Baines, K.H.; Barnes, J.W.; Griffith, C.A.; Hirtzig, M.; Pitman, K.M.; Sotin, Christophe; Brown, R.H.; Buratti, B.J.; Clark, R.N.; Nicholson, P.D.

2009-01-01

Clouds on Titan result from the condensation of methane and ethane and, as on other planets, are primarily structured by circulation of the atmosphere. At present, cloud activity mainly occurs in the southern (summer) hemisphere, arising near the pole and at mid-latitudes from cumulus updrafts triggered by surface heating and/or local methane sources, and at the north (winter) pole, resulting from the subsidence and condensation of ethane-rich air into the colder troposphere. General circulation models predict that this distribution should change with the seasons on a 15-year timescale, and that clouds should develop under certain circumstances at temperate latitudes (40??) in the winter hemisphere. The models, however, have hitherto been poorly constrained and their long-term predictions have not yet been observationally verified. Here we report that the global spatial cloud coverage on Titan is in general agreement with the models, confirming that cloud activity is mainly controlled by the global circulation. The non-detection of clouds at latitude 40??N and the persistence of the southern clouds while the southern summer is ending are, however, both contrary to predictions. This suggests that Titans equator-to-pole thermal contrast is overestimated in the models and that its atmosphere responds to the seasonal forcing with a greater inertia than expected. ?? 2009 Macmillan Publishers Limited. All rights reserved.

The impact of organic vapours on warm cloud formation; characterisation of chamber setup and first experimental results

NASA Astrophysics Data System (ADS)

Frey, Wiebke; Connolly, Paul; Dorsey, James; Hu, Dawei; Alfarra, Rami; McFiggans, Gordon

2016-04-01

The Manchester Ice Cloud Chamber (MICC), consisting of a 10m high stainless steel tube and 1m in diameter, can be used to study cloud processes. MICC is housed in three separate cold rooms stacked on top of each other and warm pseudo-adiabatic expansion from controlled initial temperature and pressure is possible through chamber evacuation. Further details about the facility can be found at http://www.cas.manchester.ac.uk/restools/cloudchamber/index.html. MICC can be connected to the Manchester Aerosol Chamber (MAC, http://www.cas.manchester.ac.uk/restools/aerosolchamber/), which allows to inject specified aerosol particles into the cloud chamber for nucleation studies. The combination of MAC and MICC will be used in the CCN-Vol project, which seeks to bring the experimental evidence for co-condensation of organic and water vapour in cloud formation which leads to an increase in cloud particle numbers (see Topping et al., 2013, Nature Geoscience Letters, for details). Here, we will show a characterisation of the cloud and aerosol chamber coupling in regard to background aerosol particles and nucleation. Furthermore, we will show preliminary results from the warm CCN-Vol experiment, investigating the impact of co-condensation of organic vapours and water vapour on warm cloud droplet formation.

Understanding Rapid Changes in Phase Partitioning between Cloud Liquid and Ice in Stratiform Mixed-Phase Clouds: An Arctic Case Study

DOE PAGES

Kalesse, Heike; de Boer, Gijs; Solomon, Amy; ...

2016-11-23

Understanding phase transitions in mixed-phase clouds is of great importance because the hydrometeor phase controls the lifetime and radiative effects of clouds. These cloud radiative effects have a crucial impact on the surface energy budget and thus on the evolution of the ice cover, in high altitudes. For a springtime low-level mixed-phase stratiform cloud case from Barrow, Alaska, a unique combination of instruments and retrieval methods is combined with multiple modeling perspectives to determine key processes that control cloud phase partitioning. The interplay of local cloud-scale versus large-scale processes is considered. Rapid changes in phase partitioning were found to bemore » caused by several main factors. Some major influences were the large-scale advection of different air masses with different aerosol concentrations and humidity content, cloud-scale processes such as a change in the thermodynamical coupling state, and local-scale dynamics influencing the residence time of ice particles. Other factors such as radiative shielding by a cirrus and the influence of the solar cycle were found to only play a minor role for the specific case study (11–12 March 2013). Furthermore, for an even better understanding of cloud phase transitions, observations of key aerosol parameters such as profiles of cloud condensation nucleus and ice nucleus concentration are desirable.« less

Understanding Rapid Changes in Phase Partitioning between Cloud Liquid and Ice in Stratiform Mixed-Phase Clouds: An Arctic Case Study

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kalesse, Heike; de Boer, Gijs; Solomon, Amy

Understanding phase transitions in mixed-phase clouds is of great importance because the hydrometeor phase controls the lifetime and radiative effects of clouds. These cloud radiative effects have a crucial impact on the surface energy budget and thus on the evolution of the ice cover, in high altitudes. For a springtime low-level mixed-phase stratiform cloud case from Barrow, Alaska, a unique combination of instruments and retrieval methods is combined with multiple modeling perspectives to determine key processes that control cloud phase partitioning. The interplay of local cloud-scale versus large-scale processes is considered. Rapid changes in phase partitioning were found to bemore » caused by several main factors. Some major influences were the large-scale advection of different air masses with different aerosol concentrations and humidity content, cloud-scale processes such as a change in the thermodynamical coupling state, and local-scale dynamics influencing the residence time of ice particles. Other factors such as radiative shielding by a cirrus and the influence of the solar cycle were found to only play a minor role for the specific case study (11–12 March 2013). Furthermore, for an even better understanding of cloud phase transitions, observations of key aerosol parameters such as profiles of cloud condensation nucleus and ice nucleus concentration are desirable.« less

Constraining the instantaneous aerosol influence on cloud albedo

DOE PAGES

Gryspeerdt, Edward; Quaas, Johannes; Ferrachat, Sylvaine; ...

2017-04-26

Much of the uncertainty in estimates of the anthropogenic forcing of climate change comes from uncertainties in the instantaneous effect of aerosols on cloud albedo, known as the Twomey effect or the radiative forcing from aerosol–cloud interactions (RFaci), a component of the total or effective radiative forcing. Because aerosols serving as cloud condensation nuclei can have a strong influence on the cloud droplet number concentration ( N d), previous studies have used the sensitivity of the N d to aerosol properties as a constraint on the strength of the RFaci. However, recent studies have suggested that relationships between aerosol andmore » cloud properties in the present-day climate may not be suitable for determining the sensitivity of the N d to anthropogenic aerosol perturbations. Using an ensemble of global aerosol–climate models, this study demonstrates how joint histograms between N d and aerosol properties can account for many of the issues raised by previous studies. It shows that if the anthropogenic contribution to the aerosol is known, the RFaci can be diagnosed to within 20% of its actual value. Furthermore, the accuracy of different aerosol proxies for diagnosing the RFaci is investigated, confirming that using the aerosol optical depth significantly underestimates the strength of the aerosol–cloud interactions in satellite data.« less

Constraining the instantaneous aerosol influence on cloud albedo

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gryspeerdt, Edward; Quaas, Johannes; Ferrachat, Sylvaine

Much of the uncertainty in estimates of the anthropogenic forcing of climate change comes from uncertainties in the instantaneous effect of aerosols on cloud albedo, known as the Twomey effect or the radiative forcing from aerosol–cloud interactions (RFaci), a component of the total or effective radiative forcing. Because aerosols serving as cloud condensation nuclei can have a strong influence on the cloud droplet number concentration ( N d), previous studies have used the sensitivity of the N d to aerosol properties as a constraint on the strength of the RFaci. However, recent studies have suggested that relationships between aerosol andmore » cloud properties in the present-day climate may not be suitable for determining the sensitivity of the N d to anthropogenic aerosol perturbations. Using an ensemble of global aerosol–climate models, this study demonstrates how joint histograms between N d and aerosol properties can account for many of the issues raised by previous studies. It shows that if the anthropogenic contribution to the aerosol is known, the RFaci can be diagnosed to within 20% of its actual value. Furthermore, the accuracy of different aerosol proxies for diagnosing the RFaci is investigated, confirming that using the aerosol optical depth significantly underestimates the strength of the aerosol–cloud interactions in satellite data.« less

Constraining the instantaneous aerosol influence on cloud albedo

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gryspeerdt, Edward; Quaas, Johannes; Ferrachat, Sylvaine

2017-04-26

Much of the uncertainty in estimates of the anthropogenic forcing of climate change comes from uncertainties in the instantaneous effect of aerosols on cloud albedo, known as the Twomey effect or the radiative forcing from aerosol–cloud interactions (RFaci), a component of the total or effective radiative forcing. Because aerosols serving as cloud condensation nuclei can have a strong influence on the cloud droplet number concentration (Nd), previous studies have used the sensitivity of the Nd to aerosol properties as a constraint on the strength of the RFaci. However, recent studies have suggested that relationships between aerosol and cloud properties inmore » the present-day climate may not be suitable for determining the sensitivity of the Nd to anthropogenic aerosol perturbations. Using an ensemble of global aerosol–climate models, this study demonstrates how joint histograms between Nd and aerosol properties can account for many of the issues raised by previous studies. It shows that if the anthropogenic contribution to the aerosol is known, the RFaci can be diagnosed to within 20% of its actual value. The accuracy of different aerosol proxies for diagnosing the RFaci is investigated, confirming that using the aerosol optical depth significantly underestimates the strength of the aerosol–cloud interactions in satellite data.« less

Constraining the instantaneous aerosol influence on cloud albedo.

PubMed

Gryspeerdt, Edward; Quaas, Johannes; Ferrachat, Sylvaine; Gettelman, Andrew; Ghan, Steven; Lohmann, Ulrike; Morrison, Hugh; Neubauer, David; Partridge, Daniel G; Stier, Philip; Takemura, Toshihiko; Wang, Hailong; Wang, Minghuai; Zhang, Kai

2017-05-09

Much of the uncertainty in estimates of the anthropogenic forcing of climate change comes from uncertainties in the instantaneous effect of aerosols on cloud albedo, known as the Twomey effect or the radiative forcing from aerosol-cloud interactions (RFaci), a component of the total or effective radiative forcing. Because aerosols serving as cloud condensation nuclei can have a strong influence on the cloud droplet number concentration ( N d ), previous studies have used the sensitivity of the N d to aerosol properties as a constraint on the strength of the RFaci. However, recent studies have suggested that relationships between aerosol and cloud properties in the present-day climate may not be suitable for determining the sensitivity of the N d to anthropogenic aerosol perturbations. Using an ensemble of global aerosol-climate models, this study demonstrates how joint histograms between N d and aerosol properties can account for many of the issues raised by previous studies. It shows that if the anthropogenic contribution to the aerosol is known, the RFaci can be diagnosed to within 20% of its actual value. The accuracy of different aerosol proxies for diagnosing the RFaci is investigated, confirming that using the aerosol optical depth significantly underestimates the strength of the aerosol-cloud interactions in satellite data.

Eulerian and Lagrangian approaches to multidimensional condensation and collection

NASA Astrophysics Data System (ADS)

Li, Xiang-Yu; Brandenburg, A.; Haugen, N. E. L.; Svensson, G.

2017-06-01

Turbulence is argued to play a crucial role in cloud droplet growth. The combined problem of turbulence and cloud droplet growth is numerically challenging. Here an Eulerian scheme based on the Smoluchowski equation is compared with two Lagrangian superparticle (or superdroplet) schemes in the presence of condensation and collection. The growth processes are studied either separately or in combination using either two-dimensional turbulence, a steady flow or just gravitational acceleration without gas flow. Good agreement between the different schemes for the time evolution of the size spectra is observed in the presence of gravity or turbulence. The Lagrangian superparticle schemes are found to be superior over the Eulerian one in terms of computational performance. However, it is shown that the use of interpolation schemes such as the cloud-in-cell algorithm is detrimental in connection with superparticle or superdroplet approaches. Furthermore, the use of symmetric over asymmetric collection schemes is shown to reduce the amount of scatter in the results. For the Eulerian scheme, gravitational collection is rather sensitive to the mass bin resolution, but not so in the case with turbulence.