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Sample records for excite luttinger liquid

  1. Fractional Josephson current through a Luttinger liquid with topological excitations

    SciTech Connect

    Wang, Rui; Wang, Baigeng Xing, D.Y.

    2015-07-15

    Recently, the Majorana fermion has received great attentions due to its promising application in the fault-tolerant quantum computation. This application requires more accessible methods to detect the motion and braiding of the Majorana fermions. We use a Luttinger liquid ring to achieve this goal, where the ring geometry is nontrivial in the sense that it leads to fermion-parity-dependent topological excitations. First, we briefly review the essential physics of the Luttinger liquid and the Majorana fermion, in order to give an introduction of the general framework used in the following main work. Then, we theoretically investigated the DC Josephson effect between two topological superconductors via a Luttinger liquid ring. A low-energy effective Hamiltonian is derived to show the existence of the fractional Josephson current. Also, we find that the amplitude of the Josephson current, which is determined by the correlation function of Luttinger liquid, exhibits different behaviors in terms of the parity of Luttinger liquid due to the topological excitations. Our results suggest a possible method to detect the Majorana fermions and their tunneling process.

  2. Excitation energy after a smooth quench in a Luttinger liquid

    SciTech Connect

    Dziarmaga, Jacek; Tylutki, Marek

    2011-12-01

    Low-energy physics of quasi-one-dimensional ultracold atomic gases is often described by a gapless Luttinger liquid (LL). It is nowadays routine to manipulate these systems by changing their parameters in time but, no matter how slow the manipulation is, it must excite a gapless system. We study a smooth change of parameters of the LL (a smooth ''quench'') with a variable quench time and find that the excitation energy decays with an inverse power of the quench time. This universal exponent is -2 at zero temperature and -1 for slow enough quenches at finite temperature. The smooth quench does not excite beyond the range of validity of the low-energy LL description.

  3. Landau's quasiparticle mapping: Fermi liquid approach and Luttinger liquid behavior.

    PubMed

    Heidbrink, Caspar P; Uhrig, Götz S

    2002-04-01

    A continuous unitary transformation is introduced which realizes Landau's mapping of the elementary excitations (quasiparticles) of an interacting Fermi liquid system to those of the system without interaction. The conservation of the number of quasiparticles is important. The transformation is performed numerically for a one-dimensional system, i.e., the worst case for a Fermi liquid approach. Yet evidence for Luttinger liquid behavior is found. Such an approach may open a route to a unified description of Fermi and Luttinger liquids on all energy scales.

  4. Kinetic theory for interacting Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Buchhold, Michael; Diehl, Sebastian

    2015-10-01

    We derive a closed set of equations for the kinetics and non-equilibrium dynamics of interacting Luttinger Liquids with cubic resonant interactions. In the presence of these interactions, the Luttinger phonons become dressed but still well defined quasi-particles, characterized by a life-time much larger then the inverse energy. This enables the separation of forward time dynamics and relative time dynamics into slow and fast dynamics and justifies the so-called Wigner approximation, which can be seen as a "local-time approximation" for the relative dynamics. Applying field theoretical methods in the Keldysh framework, i.e. kinetic and Dyson-Schwinger equations, we derive a closed set of dynamic equations, describing the kinetics of normal and anomalous phonon densities, the phonon self-energy and vertex corrections for a Gaussian non-equilibrium initial state. In the limit of low phonon densities, the results from self-consistent Born approximation are recaptured, including Andreev's scaling solution for the quasi-particle life-time in a thermal state. As an application, we compute the relaxation of an excited state to its thermal equilibrium. While the intermediate time dynamics displays exponentially fast relaxation, the last stages of thermalization are governed by algebraic laws. This can be traced back to the importance of energy and momentum conservation at the longest times, which gives rise to dynamical slow modes.

  5. Is the Luttinger Liquid a New State of Matter?

    NASA Astrophysics Data System (ADS)

    Afonin, V. V.; Petrov, V. Y.

    2010-02-01

    We are demonstrating that the Luttinger model with short range interaction can be treated as a type of Fermi liquid. In line with the main dogma of Landau’s theory one can define a fermion excitation renormalized by interaction and show that in terms of these fermions any excited state of the system is described by free particles. The fermions are a mixture of renormalized right and left electrons. The electric charge and chirality of the Landau quasi-particle is discussed.

  6. Spin Dimers: from BEC to Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Giamarchi, Thierry

    2011-03-01

    Localized spin systems, and in particular dimer systems, provide a fantastic laboratory to study the interplay between quantum effects and the interaction between excitations. Magnetic field and temperature allow an excellent control on the density of excitations and various very efficient probes such as neutrons and NMR are available. They can thus be used as ``quantum simulators'' to tackle with great success questions that one would normally search in itinerant interacting quantum systems. In particular they have provided excellent realizations of Bose-Einstein condensates [1,2]. This allowed not only to probe the properties of interacting bosons in a variety of dimensions but also to study in a controlled way additional effects such as disorder. If the dimensionality is reduced they also allow to test in a quantitative way Luttinger liquid physics [3,4,5]. I will discuss these various cases, and show that we have now good theoretical tools to make quantitative comparisons with the experiments. Finally, how to go from this low dimensional case where the spins behave essentially as fermions, to the higher dimensional case where they behave as (essentially free) bosons, is a very challenging, and experimentally relevant issue. This work was supported in part by the Swiss SNF under MaNEP and division II.

  7. Luttinger liquid with complex forward scattering: Robustness and Berry phase

    NASA Astrophysics Data System (ADS)

    Dóra, Balázs; Moessner, Roderich

    2016-02-01

    Luttinger liquids (LLs) are one-dimensional systems with well-understood instabilities due to Umklapp or backscattering. We study a generalization of the Luttinger model, which incorporates a time reversal symmetry breaking interaction producing a complex forward scattering amplitude (g2 process). The resulting low energy state is still a LL and belongs to the family of interacting Schulz-Shastry models. Remarkably, it becomes increasingly robust against additional perturbations—for purely imaginary g2, both Umklapp and local backscattering are always irrelevant. Changing the phase of the interaction generates a nontrivial Berry phase, with a universal geometric phase difference between ground and a one boson excited state depending only on the LL parameter.

  8. Compressible Strips, Chiral Luttinger Liquids, and All That Jazz

    NASA Astrophysics Data System (ADS)

    MacDonald, A. H.

    1996-03-01

    When the quantum Hall effect occurs in a two-dimensional electron gas, all low-energy elementary excitations are localized near the system edge. The edge acts in many ways like a one-dimensional ring of electrons, except that a finite current flows around the ring in equilibrium. This article is a brief and informal review of some of the physics of quantum Hall system edges. We discuss the implications of macroscopic {\\em compressible strip} models for microscopic {chiral Luttinger liquid} models and make an important distinction between the origin of non-Fermi-liquid behavior in fractional quantum Hall edges and in usual one-dimensional electron gas systems.

  9. Helical Luttinger liquid in topological insulator nanowires.

    PubMed

    Egger, R; Zazunov, A; Yeyati, A Levy

    2010-09-24

    We derive and analyze the effective low-energy theory for interacting electrons in a cylindrical nanowire made of a strong topological insulator. Three different approaches provide a consistent picture for the band structure, where surface states forming inside the bulk gap correspond to one-dimensional bands indexed by total angular momentum. When a half-integer magnetic flux pierces the nanowire, we find a strongly correlated helical Luttinger liquid topologically protected against weak disorder. We describe how transport experiments can detect this state.

  10. Brownian scattering of a spinon in a Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Rieder, M.-T.; Levchenko, A.; Micklitz, T.

    2014-12-01

    We consider strongly interacting one-dimensional electron liquids where elementary excitations carry either spin or charge. At small temperatures a spinon created at the bottom of its band scatters off low-energy spin and charge excitations and follows the diffusive motion of a Brownian particle in momentum space. We calculate the mobility characterizing these processes and show that the resulting diffusion coefficient of the spinon is parametrically enhanced at low temperatures compared to that of a mobile impurity in a spinless Luttinger liquid. We briefly discuss that this hints at the relevance of spin in the process of equilibration of strongly interacting one-dimensional electrons, and comment on implications for transport in clean single-channel quantum wires.

  11. Direct Observation of Spin- and Charge-Density Waves in a Luttinger Liquid

    NASA Astrophysics Data System (ADS)

    Cao, Chenglin; Marcum, Andrew; Mawardi Ismail, Arif; Fonta, Francisco; O'Hara, Kenneth

    2016-05-01

    At low energy, interacting fermions in one dimension (e.g. electrons in quantum wires or fermionic atoms in 1D waveguides) should behave as Luttinger liquids. In stark contrast to Fermi liquids, the low-energy elementary excitations in Luttinger liquids are collective sound-like modes that propagate independently as spin-density and/or charge-density (i.e. particle-density) waves with generally unequal, and interaction-dependent, velocities. Here we aim to unambiguously confirm this hallmark feature of the Luttinger liquid - the phenomenon of spin-charge separation - by directly observing in real space the dynamics of spin-density and ``charge''-density waves excited in an ultracold gas of spin-1/2 fermions confined in an array of 1D optical waveguides. Starting from a two-component mixture of 6 Li atoms harmonically confined along each of the 1D waveguides, we excite low lying normal modes of the trapped system - namely the spin dipole and density dipole and quadrupole modes - and measure their frequency as a function of interaction strength. Luttinger liquid theory predicts that the spin dipole frequency is strongly dependent on interaction strength whereas the density dipole and quadrupole mode frequencies are relatively insensitive. We will also discuss extending our approach to exciting localized spin density and particle density wavepackets which should propagate at different velocities. Supported by AFOSR and NSF.

  12. Universal transport dynamics in a quenched tunnel-coupled Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Gambetta, F. M.; Cavaliere, F.; Citro, R.; Sassetti, M.

    2016-07-01

    The transport dynamics of a quenched Luttinger liquid tunnel-coupled to a fermionic reservoir is investigated. In the transient dynamics, we show that for a sudden quench of the electron interaction universal power-law decay in time of the tunneling current occurs, ascribed to the presence of entangled compound excitations created by the quench. In sharp contrast to the usual nonuniversal power-law behavior of a zero-temperature nonquenched Luttinger liquid, the steady-state tunneling current is Ohmic and can be explained in terms of an effective quench-activated heating of the system. Our study unveils an unconventional dynamics for a quenched Luttinger liquid that could be identified in quenched cold Fermi gases.

  13. How to Extract Luttinger Liquid Velocity from Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Ngai, Darryl H.; Hou, Chang-Yu; Kim, Eun-Ah

    2011-03-01

    We propose direct detection of Luttinger Liquid velocity of the charge collective mode in carbon nanotubes using optical conductivity and Coulomb blockade effect. We note that detection of such fractionalized excitation needs to exploit the energy or frequency scale tied to the finite length of the nanotube. This is why previous experimental attempts have been unsuccessful. We will discuss features in the optical conductivity sensitive to the velocity of the collective mode which would be observable in the high temperature limit. In the low temperature limit, spacing between the Coulomb blockade peaks in the conductance as a function of gate voltage will be a sensitive probe. Z. Zhong et al., Nature Nanotechnology 3, 201 (2008)

  14. Incoherent scatterer in a Luttinger liquid: a new paradigmatic limit.

    PubMed

    Altland, Alexander; Gefen, Yuval; Rosenow, Bernd

    2012-03-30

    We address the problem of a Luttinger liquid with a scatterer that allows for both coherent and incoherent scattering channels. The asymptotic behavior at zero temperature is governed by a new stable fixed point: A Goldstone mode dominates the low energy dynamics, leading to universal behavior. This limit is marked by equal probabilities for forward and backward scattering. Notwithstanding this nontrivial scattering pattern, we find that the shot noise as well as cross-current correlations vanish. We thus present a paradigmatic picture of an impurity in the Luttinger model, alternative to the Kane-Fisher picture.

  15. Tunable Nonequilibrium Luttinger Liquid Based on Counterpropagating Edge Channels

    NASA Astrophysics Data System (ADS)

    Prokudina, M. G.; Ludwig, S.; Pellegrini, V.; Sorba, L.; Biasiol, G.; Khrapai, V. S.

    2014-05-01

    We investigate the energy transfer between counterpropagating quantum Hall edge channels (ECs) in a two-dimensional electron system at a filling factor of ν =1. The ECs are separated by a thin impenetrable potential barrier and Coulomb coupled, thereby constituting a quasi-one-dimensional analogue of a spinless Luttinger liquid (LL). We drive one, say hot, EC far from thermal equilibrium and measure the energy transfer rate P into the second, cold, EC using a quantum point contact as a bolometer. The dependence of P on the drive bias indicates a breakdown of the momentum conservation, whereas P is almost independent of the length of the region where the ECs interact. Interpreting our results in terms of plasmons (collective density excitations), we find that the energy transfer between the ECs occurs via plasmon backscattering at the boundaries of the LL. The backscattering probability is determined by the LL interaction parameter and can be tuned by changing the width of the electrostatic potential barrier between the ECs.

  16. Quantum Quenches in Arrays of Coupled Luttinger Liquids

    NASA Astrophysics Data System (ADS)

    James, Andrew; Hallam, Andrew; Konik, Robert; Green, Andrew

    Cold atom realisations of one dimensional interacting bosonic models are typically formed as large arrays of decoupled tubes. A low energy description of the individual tubes (including the Lieb-Liniger case) is provided by Luttinger liquid theory. Using matrix product state methods combined with integrability, we study the time evolution of an infinite array of coupled Luttinger Liquids, after a quantum quench in which interchain tunnelling is switched on to form a 2D system. We extract the time dependence of the density, bosonic modes, the Loschmidt echo and the entanglement entropy and consider possible implications for phase transitions in the coupled chain system. Our results are compared to perturbation theory and contrasted with simulations for coupled arrays of massive chains. Epsrc Grant No. EP/L010623/1 and DOE Contract No. DEAC02-98CH10886.

  17. Terahertz Spectroscopy of Individual Single-Walled Carbon Nanotubes as a Probe of Luttinger Liquid Physics.

    PubMed

    Chudow, Joel D; Santavicca, Daniel F; Prober, Daniel E

    2016-08-10

    Luttinger liquid theory predicts that collective electron excitations due to strong electron-electron interactions in a one-dimensional (1D) system will result in a modification of the collective charge-propagation velocity. By utilizing a circuit model for an individual metallic single-walled carbon nanotube as a nanotransmission line, it has been shown that the frequency-dependent terahertz impedance of a carbon nanotube can probe this expected 1D Luttinger liquid behavior. We excite terahertz standing-wave resonances on individual antenna-coupled metallic single-walled carbon nanotubes. The terahertz signal is rectified using the nanotube contact nonlinearity, allowing for a low-frequency readout of the coupled terahertz current. The charge velocity on the nanotube is determined from the terahertz spectral response. Our measurements show that a carbon nanotube can behave as a Luttinger liquid system with charge-propagation velocities that are faster than the Fermi velocity. Understanding what determines the charge velocity in low-dimensional conductors is important for the development of next generation nanodevices. PMID:27439013

  18. Terahertz Spectroscopy of Individual Single-Walled Carbon Nanotubes as a Probe of Luttinger Liquid Physics.

    PubMed

    Chudow, Joel D; Santavicca, Daniel F; Prober, Daniel E

    2016-08-10

    Luttinger liquid theory predicts that collective electron excitations due to strong electron-electron interactions in a one-dimensional (1D) system will result in a modification of the collective charge-propagation velocity. By utilizing a circuit model for an individual metallic single-walled carbon nanotube as a nanotransmission line, it has been shown that the frequency-dependent terahertz impedance of a carbon nanotube can probe this expected 1D Luttinger liquid behavior. We excite terahertz standing-wave resonances on individual antenna-coupled metallic single-walled carbon nanotubes. The terahertz signal is rectified using the nanotube contact nonlinearity, allowing for a low-frequency readout of the coupled terahertz current. The charge velocity on the nanotube is determined from the terahertz spectral response. Our measurements show that a carbon nanotube can behave as a Luttinger liquid system with charge-propagation velocities that are faster than the Fermi velocity. Understanding what determines the charge velocity in low-dimensional conductors is important for the development of next generation nanodevices.

  19. Phase transitions for a collective coordinate coupled to Luttinger liquids.

    PubMed

    Horovitz, Baruch; Giamarchi, Thierry; Le Doussal, Pierre

    2013-09-13

    We study various realizations of collective coordinates, e.g., the position of a particle, the charge of a Coulomb box, or the phase of a Bose or a superconducting condensate, coupled to Luttinger liquids with N flavors. We find that for a Luttinger parameter (1/2)

  20. Prethermalization and thermalization of a quenched interacting Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Buchhold, Michael; Heyl, Markus; Diehl, Sebastian

    2016-07-01

    We study the relaxation dynamics of interacting one-dimensional fermions with band curvature after a weak quench in the interaction parameter at zero temperature. Our model lies within the class of interacting Luttinger liquids, where the harmonic Luttinger theory is extended by a weak-integrability-breaking phonon scattering term. In order to solve for the nonequilibrium time evolution, we use quantum kinetic equations exploiting the resonant but subleading character of the phonon interaction term. The interplay between phonon scattering and the quadratic Luttinger theory leads to the emergence of three distinct spatiotemporal regimes for the fermionic real-space correlation function. It features the crossover from a prequench to a prethermal state, finally evolving towards a thermal state on increasing length and time scales. The characteristic algebraically decaying real-space correlations in the prethermalized regime become modulated by an amplitude that is decaying in time according to a stretched exponential as an effect of the interactions. The asymptotic thermalization dynamics is governed by energy transport over large distances from the thermalized to the nonthermalized regions via macroscopic, dynamical slow modes. This is revealed in an algebraic decay of the system's effective temperature. The numerical value of the associated exponent agrees with the dynamical critical exponent of the Kardar-Parisi-Zhang universality class. We also discuss a criterion for the applicability of this theory away from the integrable limit of noninteracting fermions.

  1. Plasmon decay and thermal transport from spin-charge coupling in generic Luttinger liquids.

    PubMed

    Levchenko, Alex

    2014-11-01

    We discuss the violation of spin-charge separation in generic nonlinear Luttinger liquids and investigate its effect on the relaxation and thermal transport of genuine spin-1/2 electron liquids in ballistic quantum wires. We identify basic scattering processes compatible with the symmetry of the problem and conservation laws that lead to the decay of plasmons into the spin modes. We derive a closed set of coupled kinetic equations for the spin-charge excitations and solve the problem of thermal conductance of interacting electrons for an arbitrary relation between the quantum wire length and spin-charge thermalization length. PMID:25415912

  2. Plasmon Decay and Thermal Transport from Spin-Charge Coupling in Generic Luttinger Liquids

    NASA Astrophysics Data System (ADS)

    Levchenko, Alex

    2014-11-01

    We discuss the violation of spin-charge separation in generic nonlinear Luttinger liquids and investigate its effect on the relaxation and thermal transport of genuine spin-1 /2 electron liquids in ballistic quantum wires. We identify basic scattering processes compatible with the symmetry of the problem and conservation laws that lead to the decay of plasmons into the spin modes. We derive a closed set of coupled kinetic equations for the spin-charge excitations and solve the problem of thermal conductance of interacting electrons for an arbitrary relation between the quantum wire length and spin-charge thermalization length.

  3. Coherence and Localization in 2D Luttinger Liquids

    SciTech Connect

    Anderson, P.W.; Ramakrishnan, T.V.; Strong, S.; Clarke, D.G. |||

    1996-11-01

    Recent measurements on the resistivity of (La-Sr){sub 2}CuO{sub 4} are shown to fit within the general framework of Luttinger liquid transport theory. They exhibit a crossover from the spin-charge separated {open_quote}{open_quote}holon nondrag regime{close_quote}{close_quote} usually observed, with {rho}{sub {ital ab}}{approximately}{ital T}, to a {open_quote}{open_quote}localizing{close_quote}{close_quote} regime dominated by impurity scattering at low temperature. The proportionality of {rho}{sub {ital c}} and {rho}{sub {ital ab}} and the giant anisotropy follow directly from the theory. {copyright} {ital 1996 The American Physical Society.}

  4. Reprint of : Measuring the Luttinger liquid parameter with shot noise

    NASA Astrophysics Data System (ADS)

    Kühne, J. K.; Protopopov, I. V.; Oreg, Y.; Mirlin, A. D.

    2016-08-01

    We explore the low-frequency noise of interacting electrons in a one-dimensional structure (quantum wire or interaction-coupled edge states) with counterpropagating modes, assuming a single channel in each direction. The system is driven out of equilibrium by a quantum point contact (QPC) with an applied voltage, which induces a double-step energy distribution of incoming electrons on one side of the device. A second QPC serves to explore the statistics of outgoing electrons. We show that measurement of a low-frequency noise in such a setup allows one to extract the Luttinger liquid constant K which is the key parameter characterizing an interacting 1D system. We evaluate the dependence of the zero-frequency noise on K and on parameters of both QPCs (transparencies and voltages).

  5. Luttinger Liquid, Singular Interaction and Quantum Criticality in Cuprate Materials

    NASA Astrophysics Data System (ADS)

    di Castro, C.; Caprara, S.

    2014-10-01

    With particular reference to the role of the renormalization group (RG) approach and Ward identities (WI's), we start by recalling some old features of the one-dimensional Luttinger liquid as the prototype of non-Fermi-liquid behavior. Its dimensional crossover to the Landau normal Fermi liquid implies that a non-Fermi liquid, as, e.g., the normal phase of the cuprate high temperature superconductors, can be maintained in d > 1 only in the presence of a sufficiently singular effective interaction among the charge carriers. This is the case when, nearby an instability, the interaction is mediated by critical fluctuations. We are then led to introduce the specific case of superconductivity in cuprates as an example of avoided quantum criticality. We will disentangle the fluctuations which act as mediators of singular electron-electron interaction, enlightening the possible order competing with superconductivity and a mechanism for the non-Fermi-liquid behavior of the metallic phase. This paper is not meant to be a comprehensive review. Many important contributions will not be considered. We will also avoid using extensive technicalities and making full calculations for which we refer to the original papers and to the many good available reviews. We will here only follow one line of reasoning which guided our research activity in this field.

  6. One-Dimensional Liquid ^{4}He: Dynamical Properties beyond Luttinger-Liquid Theory.

    PubMed

    Bertaina, G; Motta, M; Rossi, M; Vitali, E; Galli, D E

    2016-04-01

    We compute the zero-temperature dynamical structure factor of one-dimensional liquid ^{4}He by means of state-of-the-art quantum Monte Carlo and analytic continuation techniques. By increasing the density, the dynamical structure factor reveals a transition from a highly compressible critical liquid to a quasisolid regime. In the low-energy limit, the dynamical structure factor can be described by the quantum hydrodynamic Luttinger-liquid theory, with a Luttinger parameter spanning all possible values by increasing the density. At higher energies, our approach provides quantitative results beyond the Luttinger-liquid theory. In particular, as the density increases, the interplay between dimensionality and interaction makes the dynamical structure factor manifest a pseudo-particle-hole continuum typical of fermionic systems. At the low-energy boundary of such a region and moderate densities, we find consistency, within statistical uncertainties, with predictions of a power-law structure by the recently developed nonlinear Luttinger-liquid theory. In the quasisolid regime, we observe a novel behavior at intermediate momenta, which can be described by new analytical relations that we derive for the hard-rods model. PMID:27081985

  7. One-Dimensional Liquid ^{4}He: Dynamical Properties beyond Luttinger-Liquid Theory.

    PubMed

    Bertaina, G; Motta, M; Rossi, M; Vitali, E; Galli, D E

    2016-04-01

    We compute the zero-temperature dynamical structure factor of one-dimensional liquid ^{4}He by means of state-of-the-art quantum Monte Carlo and analytic continuation techniques. By increasing the density, the dynamical structure factor reveals a transition from a highly compressible critical liquid to a quasisolid regime. In the low-energy limit, the dynamical structure factor can be described by the quantum hydrodynamic Luttinger-liquid theory, with a Luttinger parameter spanning all possible values by increasing the density. At higher energies, our approach provides quantitative results beyond the Luttinger-liquid theory. In particular, as the density increases, the interplay between dimensionality and interaction makes the dynamical structure factor manifest a pseudo-particle-hole continuum typical of fermionic systems. At the low-energy boundary of such a region and moderate densities, we find consistency, within statistical uncertainties, with predictions of a power-law structure by the recently developed nonlinear Luttinger-liquid theory. In the quasisolid regime, we observe a novel behavior at intermediate momenta, which can be described by new analytical relations that we derive for the hard-rods model.

  8. Spin ladders and quantum simulators for Tomonaga-Luttinger liquids.

    PubMed

    Ward, S; Bouillot, P; Ryll, H; Kiefer, K; Krämer, K W; Rüegg, Ch; Kollath, C; Giamarchi, T

    2013-01-01

    Magnetic insulators have proven to be usable as quantum simulators for itinerant interacting quantum systems. In particular the compound (C(5)H(12)N)(2)CuBr(4) (for short: (Hpip)(2)CuBr(4)) was shown to be a remarkable realization of a Tomonaga-Luttinger liquid (TLL) and allowed us to quantitatively test the TLL theory. Substitution weakly disorders this class of compounds and thus allows us to use them to tackle questions pertaining to the effect of disorder in TLL as well, such as that of the formation of the Bose glass. In this paper we present, as a first step in this direction, a study of the properties of the related (Hpip)(2)CuCl(4) compound. We determine the exchange couplings and compute the temperature and magnetic field dependence of the specific heat, using a finite temperature density matrix renormalization group procedure. Comparison with the measured specific heat at zero magnetic field confirms the exchange parameters and Hamiltonian for the (Hpip)(2)CuCl(4) compound, giving the basis needed to begin studying the disorder effects.

  9. Spin ladders and quantum simulators for Tomonaga-Luttinger liquids.

    PubMed

    Ward, S; Bouillot, P; Ryll, H; Kiefer, K; Krämer, K W; Rüegg, Ch; Kollath, C; Giamarchi, T

    2013-01-01

    Magnetic insulators have proven to be usable as quantum simulators for itinerant interacting quantum systems. In particular the compound (C(5)H(12)N)(2)CuBr(4) (for short: (Hpip)(2)CuBr(4)) was shown to be a remarkable realization of a Tomonaga-Luttinger liquid (TLL) and allowed us to quantitatively test the TLL theory. Substitution weakly disorders this class of compounds and thus allows us to use them to tackle questions pertaining to the effect of disorder in TLL as well, such as that of the formation of the Bose glass. In this paper we present, as a first step in this direction, a study of the properties of the related (Hpip)(2)CuCl(4) compound. We determine the exchange couplings and compute the temperature and magnetic field dependence of the specific heat, using a finite temperature density matrix renormalization group procedure. Comparison with the measured specific heat at zero magnetic field confirms the exchange parameters and Hamiltonian for the (Hpip)(2)CuCl(4) compound, giving the basis needed to begin studying the disorder effects. PMID:23221064

  10. Momentum-Space Entanglement and Loschmidt Echo in Luttinger Liquids after a Quantum Quench.

    PubMed

    Dóra, Balázs; Lundgren, Rex; Selover, Mark; Pollmann, Frank

    2016-07-01

    Luttinger liquids (LLs) arise by coupling left- and right-moving particles through interactions in one dimension. This most natural partitioning of LLs is investigated by the momentum-space entanglement after a quantum quench using analytical and numerical methods. We show that the momentum-space entanglement spectrum of a LL possesses many universal features both in equilibrium and after a quantum quench. The largest entanglement eigenvalue is identical to the Loschmidt echo, i.e., the overlap of the disentangled and final wave functions of the system. The second largest eigenvalue is the overlap of the first excited state of the disentangled system with zero total momentum and the final wave function. The entanglement gap is universal both in equilibrium and after a quantum quench. The momentum-space entanglement entropy is always extensive and saturates fast to a time independent value after the quench, in sharp contrast to a spatial bipartitioning.

  11. Momentum-Space Entanglement and Loschmidt Echo in Luttinger Liquids after a Quantum Quench

    NASA Astrophysics Data System (ADS)

    Dóra, Balázs; Lundgren, Rex; Selover, Mark; Pollmann, Frank

    2016-07-01

    Luttinger liquids (LLs) arise by coupling left- and right-moving particles through interactions in one dimension. This most natural partitioning of LLs is investigated by the momentum-space entanglement after a quantum quench using analytical and numerical methods. We show that the momentum-space entanglement spectrum of a LL possesses many universal features both in equilibrium and after a quantum quench. The largest entanglement eigenvalue is identical to the Loschmidt echo, i.e., the overlap of the disentangled and final wave functions of the system. The second largest eigenvalue is the overlap of the first excited state of the disentangled system with zero total momentum and the final wave function. The entanglement gap is universal both in equilibrium and after a quantum quench. The momentum-space entanglement entropy is always extensive and saturates fast to a time independent value after the quench, in sharp contrast to a spatial bipartitioning.

  12. Momentum-Space Entanglement and Loschmidt Echo in Luttinger Liquids after a Quantum Quench.

    PubMed

    Dóra, Balázs; Lundgren, Rex; Selover, Mark; Pollmann, Frank

    2016-07-01

    Luttinger liquids (LLs) arise by coupling left- and right-moving particles through interactions in one dimension. This most natural partitioning of LLs is investigated by the momentum-space entanglement after a quantum quench using analytical and numerical methods. We show that the momentum-space entanglement spectrum of a LL possesses many universal features both in equilibrium and after a quantum quench. The largest entanglement eigenvalue is identical to the Loschmidt echo, i.e., the overlap of the disentangled and final wave functions of the system. The second largest eigenvalue is the overlap of the first excited state of the disentangled system with zero total momentum and the final wave function. The entanglement gap is universal both in equilibrium and after a quantum quench. The momentum-space entanglement entropy is always extensive and saturates fast to a time independent value after the quench, in sharp contrast to a spatial bipartitioning. PMID:27419554

  13. Spin Gap and Luttinger Liquid Description of the NMR Relaxation in Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Dóra, Balázs; Gulácsi, Miklós; Simon, Ferenc; Kuzmany, Hans

    2007-10-01

    Recent NMR experiments by Singer et al. [Singer , Phys. Rev. Lett. 95, 236403 (2005).PRLTAO0031-900710.1103/PhysRevLett.95.236403] showed a deviation from Fermi-liquid behavior in carbon nanotubes with an energy gap evident at low temperatures. Here, a comprehensive theory for the magnetic field and temperature dependent NMR C13 spin-lattice relaxation is given in the framework of the Tomonaga-Luttinger liquid. The low temperature properties are governed by a gapped relaxation due to a spin gap (˜30K), which crosses over smoothly to the Luttinger liquid behavior with increasing temperature.

  14. Emergent ``super-solitons'' following an interaction strength quantum quench across a Luttinger liquid-Mott insulating phase boundary

    NASA Astrophysics Data System (ADS)

    Foster, Matthew; Yuzbashyan, Emil

    2010-03-01

    Rapid progress in cold atom experiments has motivated the study of non-equilibrium many-body dynamics following a sudden deformation of the system Hamiltonian (a ``quantum quench''). Here, we consider the dynamics of localized excitations produced via a quench across a quantum phase boundary separating critical Luttinger liquid and gapped Mott insulating states. Our initial liquid ground state is labeled by a Luttinger interaction parameter K, and subject to a density-inhomogeneity forming external potential. For the Mott insulator, we employ the quantum Sine Gordon model at the Luther-Emery (LE) point. We find that over a wide range of initial K values, the quench induces the production of relativistic, non-dispersive traveling density waves, which we dub ``super-solitons.'' The super-solitons are generated from generic antecedent localized density lumps, and appear to be a robust feature of the post-quench dynamics. An isolated exception occurs for the case of K = KLE; here, the density dynamics are generically dispersive, and depend sensitively upon the shape of the initial inhomogeneity. We show that the super-solitons do not interact, and we demonstrate that an inhomogeneous Luttinger parameter K can be used to produce super-solitons with different characteristics in the same system.

  15. Reprint of : Transient dynamics of spin-polarized injection in helical Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Calzona, A.; Carrega, M.; Dolcetto, G.; Sassetti, M.

    2016-08-01

    We analyze the time evolution of spin-polarized electron wave packets injected into the edge states of a two-dimensional topological insulator. In the presence of electron interactions, the system is described as a helical Luttinger liquid and injected electrons fractionalize. However, because of the presence of metallic detectors, no evidences of fractionalization are encoded in dc measurements, and in this regime the system does not show deviations from its non-interacting behavior. Nevertheless, we show that the helical Luttinger liquid nature emerges in the transient dynamics, where signatures of charge/spin fractionalization can be clearly identified.

  16. ESR modes in a Strong-Leg Ladder in the Tomonaga-Luttinger Liquid Phase

    NASA Astrophysics Data System (ADS)

    Zvyagin, S.; Ozerov, M.; Maksymenko, M.; Wosnitza, J.; Honecker, A.; Landee, C. P.; Turnbull, M.; Furuya, S. C.; Giamarchi, T.

    Magnetic excitations in the strong-leg quantum spin ladder compound (C7H10N)2CuBr4 (known as DIMPY) in the field-induced Tomonaga-Luttinger spin liquid phase are studied by means of high-field electron spin resonance (ESR) spectroscopy. The presence of a gapped ESR mode with unusual non-linear frequency-field dependence is revealed experimentally. Using a combination of analytic and exact diagonalization methods, we compute the dynamical structure factor and identify this mode with longitudinal excitations in the antisymmetric channel. We argue that these excitations constitute a fingerprint of the spin dynamics in a strong-leg spin-1/2 Heisenberg antiferromagnetic ladder and owe its ESR observability to the uniform Dzyaloshinskii-Moriya interaction. This work was partially supported by the DFG and Helmholtz Gemeinschaft (Germany), Swiss SNF under Division II, and ERC synergy UQUAM project. We acknowledge the support of the HLD at HZDR, member of the European Magnetic Field Laboratory (EMFL).

  17. One-dimensional quantum liquids with power-law interactions: the Luttinger staircase.

    PubMed

    Dalmonte, M; Pupillo, G; Zoller, P

    2010-10-01

    We study one-dimensional fermionic and bosonic gases with repulsive power-law interactions 1/|x|(β), with β>1, in the framework of Tomonaga-Luttinger liquid (TLL) theory. We obtain an accurate analytical expression linking the TLL parameter to the microscopic Hamiltonian, for arbitrary β and strength of the interactions. In the presence of a small periodic potential, power-law interactions make the TLL unstable towards the formation of a cascade of lattice solids with fractional filling, a "Luttinger staircase." Several of these quantum phases and phase transitions are realized with ground state polar molecules and weakly bound magnetic Feshbach molecules.

  18. One-Dimensional Quantum Liquids with Power-Law Interactions: The Luttinger Staircase

    SciTech Connect

    Dalmonte, M.; Pupillo, G.; Zoller, P.

    2010-10-01

    We study one-dimensional fermionic and bosonic gases with repulsive power-law interactions 1/|x|{sup {beta}}, with {beta}>1, in the framework of Tomonaga-Luttinger liquid (TLL) theory. We obtain an accurate analytical expression linking the TLL parameter to the microscopic Hamiltonian, for arbitrary {beta} and strength of the interactions. In the presence of a small periodic potential, power-law interactions make the TLL unstable towards the formation of a cascade of lattice solids with fractional filling, a 'Luttinger staircase'. Several of these quantum phases and phase transitions are realized with ground state polar molecules and weakly bound magnetic Feshbach molecules.

  19. Spin-incoherent one-dimensional spin-1 Bose Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Jen, H. H.; Yip, S.-K.

    2016-09-01

    We investigate spin-incoherent Luttinger liquid of a one-dimensional spin-1 Bose gas in a harmonic trap. In this regime highly degenerate spin configurations emerge since the energy splitting between different spin states is much less than the thermal energy of the system, while the temperature is low enough that the lowest energetic orbitals are occupied. As an example we numerically study the momentum distribution of a one-dimensional spin-1 Bose gas in Tonks-Girardeau gas limit and in the sector of zero magnetization. We find that the momentum distributions broaden as the number of atoms increase due to the averaging of spin function overlaps. Large momentum (p ) asymptotic is analytically derived, showing the universal 1 /p4 dependence. We demonstrate that the spin-incoherent Luttinger liquid has a momentum distribution also distinct from spinless bosons at finite temperature.

  20. Local spectral properties of Luttinger liquids: scaling versus nonuniversal energy scales

    NASA Astrophysics Data System (ADS)

    Schuricht, D.; Andergassen, S.; Meden, V.

    2013-01-01

    Motivated by recent scanning tunneling and photoemission spectroscopy measurements on self-organized gold chains on a germanium surface, we reinvestigate the local single-particle spectral properties of Luttinger liquids. In the first part we use the bosonization approach to exactly compute the local spectral function of a simplified field theoretical low-energy model and take a closer look at scaling properties as a function of the ratio of energy and temperature. Translational-invariant Luttinger liquids as well as those with an open boundary (cut chain geometry) are considered. We explicitly show that the scaling functions of both set-ups have the same analytical form. The scaling behavior suggests a variety of consistency checks which can be performed on measured data to experimentally verify Luttinger liquid behavior. In the second part we approximately compute the local spectral function of a microscopic lattice model—the extended Hubbard model—close to an open boundary using the functional renormalization group. We show that it follows the field theoretical prediction in the low-energy regime as a function of energy and temperature, and point out the importance of nonuniversal energy scales inherent to any microscopic model. The spatial dependence of this spectral function is characterized by oscillatory behavior and an envelope function which follows a power law in accordance with the field theoretical continuum model. Interestingly, for the lattice model we find a phase shift which is proportional to the two-particle interaction and not accounted for in the standard bosonization approach to Luttinger liquids with an open boundary. We briefly comment on the effects of several one-dimensional branches cutting the Fermi energy and Rashba spin-orbit interaction.

  1. Tunneling spectroscopy of a spiral Luttinger liquid in contact with superconductors

    NASA Astrophysics Data System (ADS)

    Liu, Dong E.; Levchenko, Alex

    2014-03-01

    One-dimensional wires with Rashba spin-orbit coupling, magnetic field, and strong electron-electron interactions are described by a spiral Luttinger liquid model. We develop a theory to investigate the tunneling density of states into a spiral Luttinger liquid in contact with superconductors at its two ends. This approach provides a way to disentangle the delicate interplay between superconducting correlations and strong electron interactions. If the wire-superconductor boundary is dominated by Andreev reflection, we find that in the vicinity of the interface the zero-bias tunneling anomaly reveals a power law enhancement with the unusual exponent. This zero-bias due to Andreev reflections may coexist and thus mask possible peak due to Majorana bound states. Far away from the interface strong correlations inherent to the Luttinger liquid prevail and restore conventional suppression of the tunneling density of states at the Fermi level, which acquires a Friedel-like oscillatory envelope with the period renormalized by the strength of the interaction. D.E.L. was supported by Michigan State University and in part by ARO through Contract No. W911NF-12-1-0235. A.L. acknowledges support from NSF under Grant No. PHYS-1066293, and the hospitality of the Aspen Center for Physics.

  2. Universal transport signatures of Majorana fermions in superconductor-Luttinger liquid junctions

    NASA Astrophysics Data System (ADS)

    Fidkowski, Lukasz; Alicea, Jason; Lindner, Netanel H.; Lutchyn, Roman M.; Fisher, Matthew P. A.

    2012-06-01

    One of the most promising proposals for engineering topological superconductivity and Majorana fermions employs a spin-orbit coupled nanowire subjected to a magnetic field and proximate to an s-wave superconductor. When only part of the wire's length contacts to the superconductor, the remaining conducting portion serves as a natural lead that can be used to probe these Majorana modes via tunneling. The enhanced role of interactions in one dimension dictates that this configuration should be viewed as a superconductor-Luttinger liquid junction. We investigate such junctions between both helical and spinful Luttinger liquids, and topological as well as nontopological superconductors. We determine the phase diagram for each case and show that universal low-energy transport in these systems is governed by fixed points describing either perfect normal reflection or perfect Andreev reflection. In addition to capturing (in some instances) the familiar Majorana-mediated “zero-bias anomaly” in a new framework, we show that interactions yield dramatic consequences in certain regimes. Indeed, we establish that strong repulsion removes this conductance anomaly altogether while strong attraction produces dynamically generated effective Majorana modes even in a junction with a trivial superconductor. Interactions further lead to striking signatures in the local density of states and the line shape of the conductance peak at finite voltage, and also are essential for establishing smoking-gun transport signatures of Majorana fermions in spinful Luttinger liquid junctions.

  3. Intermediate fixed point in a Luttinger liquid with elastic and dissipative backscattering

    NASA Astrophysics Data System (ADS)

    Altland, Alexander; Gefen, Yuval; Rosenow, Bernd

    2015-08-01

    In a recent work [A. Altland, Y. Gefen, and B. Rosenow, Phys. Rev. Lett. 108, 136401 (2012), 10.1103/PhysRevLett.108.136401], we have addressed the problem of a Luttinger liquid with a scatterer that allows for both coherent and incoherent scattering channels. We have found that the physics associated with this model is qualitatively different from the elastic impurity setup analyzed by Kane and Fisher, and from the inelastic scattering scenario studied by Furusaki and Matveev, thus proposing a paradigmatic picture of Luttinger liquid with an impurity. Here we present an extensive study of the renormalization group flows for this problem, the fixed point landscape, and scaling near those fixed points. Our analysis is nonperturbative in the elastic tunneling amplitudes, employing an instanton calculation in one or two of the available elastic tunneling channels. Our analysis accounts for nontrivial Klein factors, which represent anyonic or fermionic statistics. These Klein factors need to be taken into account due to the fact that higher-order tunneling processes take place. In particular, we find a stable fixed point, where an incoming current is split 1/2 -1/2 between a forward and a backward scattered beams. This intermediate fixed point, between complete backscattering and full forward scattering, is stable for the Luttinger parameter g <1 .

  4. Density functionals not based on the electron gas: local-density approximation for a Luttinger liquid.

    PubMed

    Lima, N A; Silva, M F; Oliveira, L N; Capelle, K

    2003-04-11

    By shifting the reference system for the local-density approximation (LDA) from the electron gas to other model systems, one obtains a new class of density functionals, which by design account for the correlations present in the chosen reference system. This strategy is illustrated by constructing an explicit LDA for the one-dimensional Hubbard model. While the traditional ab initio LDA is based on a Fermi liquid (the three-dimensional interacting electron gas), this one is based on a Luttinger liquid. First applications to inhomogeneous Hubbard models, including one containing a localized impurity, are reported.

  5. Density functionals not based on the electron gas: local-density approximation for a Luttinger liquid.

    PubMed

    Lima, N A; Silva, M F; Oliveira, L N; Capelle, K

    2003-04-11

    By shifting the reference system for the local-density approximation (LDA) from the electron gas to other model systems, one obtains a new class of density functionals, which by design account for the correlations present in the chosen reference system. This strategy is illustrated by constructing an explicit LDA for the one-dimensional Hubbard model. While the traditional ab initio LDA is based on a Fermi liquid (the three-dimensional interacting electron gas), this one is based on a Luttinger liquid. First applications to inhomogeneous Hubbard models, including one containing a localized impurity, are reported. PMID:12731934

  6. Cold atoms in one-dimensional rings: a Luttinger liquid approach to precision measurement

    NASA Astrophysics Data System (ADS)

    Ragole, Stephen; Taylor, Jacob

    Recent experiments have realized ring shaped traps for ultracold atoms. We consider the one-dimensional limit of these ring systems with a moving weak barrier, such as a blue-detuned laser beam. In this limit, we employ Luttinger liquid theory and find an analogy with the superconducting charge qubit. In particular, we find that strongly-interacting atoms in such a system could be used for precision rotation sensing. We compare the performance of this new sensor to the state of the art non-interacting atom interferometry. Funding provided by the Physics Frontier Center at the JQI and by DARPA QUASAR.

  7. Spin incoherent effects in momentum resolved tunneling, transport, and Coulomb drag in Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Fiete, Gregory

    2006-03-01

    In a one dimensional electron gas at low enough density the magnetic exchange energy J between neighboring electrons is exponentially suppressed relative to the Fermi energy, EF. At finite temperature T, the energy hierarchy J << T << EF can be reached, and we refer to this as the spin incoherent (SI) Luttinger liquid state. By using a model of a fluctuating Wigner solid, we theoretically explore the signatures of spin incoherence in the single particle Green’s function[1], momentum resolved tunneling[2], transport[3], and Coulomb drag[4]. In the SI Green’s function the spin modes of a Luttinger liquid (LL) are thermally washed out leaving only singular behavior from the charge modes. The charge modes are broadened in momentum space by an amount of order kF and the energy dependence of the tunneling density of states qualitatively changes from the low energy suppression of the LL regime to a possible low energy divergence in the SI regime. Such a state may be probed directly in momentum resolved tunneling between parallel quantum wires. Deep in the SI regime, the physics of transport and Coulomb drag can be mapped onto spinless electrons. Various crossovers in temperature and for finite systems connected to Fermi liquid leads are discussed. Both transport and Coulomb drag may exhibit interesting non-monotonic temperature dependence. [1] G. A. Fiete and L. Balents, Phys. Rev. Lett. 93, 226401 (2004). [2] G. A. Fiete, J. Qian, Y. Tserkovnyak, and B. I. Halperin, Phys. Rev. B 72, 045315 (2005). [3] G. A. Fiete, K. Le Hur, and L. Balents, Phys. Rev. B 72, 125416 (2005). [4] G. A. Fiete, K. Le Hur, and L. Balents, Submitted, cond-mat/0511715.

  8. The connection between spin-charge separation and hidden order in Luttinger liquids

    NASA Astrophysics Data System (ADS)

    McCulloch, Ian; Kruis, Herman; Nussinov, Zohar; Zaanen, Jan

    2004-03-01

    We demonstrate that Luttinger liquids are characterized by a form of hidden order which is similar, but distinct in some crucial regards, to the hidden order characterizing spin-1 Heisenberg chains. Following on from the well-known Ogata-Shiba factorization of the wavefunction of the strong coupling limit of the Hubbard model into pure charge (effective spinless fermions) and spin (spin-1/2 Heisenberg antiferromagnet) parts, we show that the essential geometrical construct, namely the 'squeezed space' belonging to the spin degrees of freedom, is unversal and exists even in the non-interacting fermion gas. We construct string correlation functions that probe directly the squeezed space, thereby showing how the two-point correlators factorize into spin-only and charge-only components.

  9. Dichotomy between Attractive and Repulsive Tomonaga-Luttinger Liquids in Spin Ladders.

    PubMed

    Jeong, M; Schmidiger, D; Mayaffre, H; Klanjšek, M; Berthier, C; Knafo, W; Ballon, G; Vignolle, B; Krämer, S; Zheludev, A; Horvatić, M

    2016-09-01

    We present a direct NMR method to determine whether the interactions in a Tomonaga-Luttinger liquid (TLL) state of a spin-1/2 Heisenberg antiferromagnetic ladder are attractive or repulsive. For the strong-leg spin ladder compound (C_{7}H_{10}N)_{2}CuBr_{4} we find that the isothermal magnetic field dependence of the NMR relaxation rate T_{1}^{-1}(H) displays a concave curve between the two critical fields bounding the TLL regime. This is in sharp contrast to the convex curve previously reported for a strong-rung ladder, (C_{5}H_{12}N)_{2}CuBr_{4}. We show that the concavity and the convexity of T_{1}^{-1}(H), which is a fingerprint of spin fluctuations, directly reflect the attractive and repulsive fermionic interactions in the TLL, respectively. The interaction sign is alternatively determined from an indirect method combining bulk magnetization and specific heat data. PMID:27636483

  10. Long-lived binary tunneling spectrum in the quantum Hall Tomonaga-Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Washio, K.; Nakazawa, R.; Hashisaka, M.; Muraki, K.; Tokura, Y.; Fujisawa, T.

    2016-02-01

    The existence of long-lived nonequilibrium states without showing thermalization, which has previously been demonstrated in time evolution of ultracold atoms, suggests the possibility of their spatial analog in transport behavior of interacting electrons in solid-state systems. Here we report long-lived nonequilibrium states in one-dimensional edge channels in the integer quantum Hall regime. An indirect heating scheme in a counterpropagating configuration is employed to generate a nontrivial binary spectrum consisting of high- and low-temperature components. This unusual spectrum is sustained even after traveling 5-10 μ m , much longer than the length for electronic relaxation (about 0.1 μ m ), without showing significant thermalization. This observation is consistent with the integrable model of Tomonaga-Luttinger liquid. The long-lived spectrum implies that the system is well described by noninteracting plasmons, which are attractive for carrying information for a long distance.

  11. Approaching many-body localization from disordered Luttinger liquids via the functional renormalization group

    NASA Astrophysics Data System (ADS)

    Karrasch, C.; Moore, J. E.

    2015-09-01

    We study the interplay of interactions and disorder in a one-dimensional fermion lattice coupled adiabatically to infinite reservoirs. We employ both the functional renormalization group (FRG) as well as matrix product state techniques, which serve as an accurate benchmark for small systems. Using the FRG, we compute the length- and temperature-dependence of the conductance averaged over 104 samples for lattices as large as 105 sites. We identify regimes in which non-Ohmic power law behavior can be observed and demonstrate that the corresponding exponents can be understood by adapting earlier predictions obtained perturbatively for disordered Luttinger liquids. In the presence of both disorder and isolated impurities, the conductance has a universal single-parameter scaling form. This lays the groundwork for an application of the functional renormalization group to the realm of many-body localization.

  12. Surface Tomonaga-Luttinger-Liquid State on Bi/InSb(001).

    PubMed

    Ohtsubo, Yoshiyuki; Kishi, Jun-Ichiro; Hagiwara, Kenta; Le Fèvre, Patrick; Bertran, François; Taleb-Ibrahimi, Amina; Yamane, Hiroyuki; Ideta, Shin-Ichiro; Matsunami, Masaharu; Tanaka, Kiyohisa; Kimura, Shin-Ichi

    2015-12-18

    A 1D metallic surface state was created on an anisotropic InSb(001) surface covered with Bi. Angle-resolved photoelectron spectroscopy (ARPES) showed a 1D Fermi contour with almost no 2D distortion. Close to the Fermi level (E_{F}), the angle-integrated photoelectron spectra showed power-law scaling with the binding energy and temperature. The ARPES plot above E_{F}, obtained thanks to a thermally broadened Fermi edge at room temperature, showed a 1D state with continuous metallic dispersion across E_{F} and power-law intensity suppression around E_{F}. These results strongly suggest a Tomonaga-Luttinger liquid on the Bi/InSb(001) surface. PMID:26722934

  13. Dichotomy between Attractive and Repulsive Tomonaga-Luttinger Liquids in Spin Ladders.

    PubMed

    Jeong, M; Schmidiger, D; Mayaffre, H; Klanjšek, M; Berthier, C; Knafo, W; Ballon, G; Vignolle, B; Krämer, S; Zheludev, A; Horvatić, M

    2016-09-01

    We present a direct NMR method to determine whether the interactions in a Tomonaga-Luttinger liquid (TLL) state of a spin-1/2 Heisenberg antiferromagnetic ladder are attractive or repulsive. For the strong-leg spin ladder compound (C_{7}H_{10}N)_{2}CuBr_{4} we find that the isothermal magnetic field dependence of the NMR relaxation rate T_{1}^{-1}(H) displays a concave curve between the two critical fields bounding the TLL regime. This is in sharp contrast to the convex curve previously reported for a strong-rung ladder, (C_{5}H_{12}N)_{2}CuBr_{4}. We show that the concavity and the convexity of T_{1}^{-1}(H), which is a fingerprint of spin fluctuations, directly reflect the attractive and repulsive fermionic interactions in the TLL, respectively. The interaction sign is alternatively determined from an indirect method combining bulk magnetization and specific heat data.

  14. Quantum impurity in a Luttinger liquid: Exact solution of the Kane-Fisher model

    NASA Astrophysics Data System (ADS)

    Rylands, Colin; Andrei, Natan

    2016-09-01

    A Luttinger liquid coupled to a quantum impurity describes a large number of physical systems. The Hamiltonian consists of left- and right-moving fermions interacting among themselves via a density-density coupling and scattering off a localized transmitting and reflecting impurity. We solve exactly the Hamiltonian by means of an incoming-outgoing scattering Bethe basis which properly incorporates all scattering processes. A related model, the weak-tunneling model, wherein the impurity is replaced by a tunnel junction, is solved by the same method. The consistency of the construction is established through a generalized Yang-Baxter relation. Periodic boundary conditions are imposed and the resulting Bethe ansatz equations are derived by means of the off-diagonal Bethe ansatz approach. We derive the spectrum of the model for all coupling constant regimes and calculate the impurity free energy. We discuss the low energy behavior of the systems for both repulsive and attractive interactions.

  15. Dichotomy between Attractive and Repulsive Tomonaga-Luttinger Liquids in Spin Ladders

    NASA Astrophysics Data System (ADS)

    Jeong, M.; Schmidiger, D.; Mayaffre, H.; Klanjšek, M.; Berthier, C.; Knafo, W.; Ballon, G.; Vignolle, B.; Krämer, S.; Zheludev, A.; Horvatić, M.

    2016-09-01

    We present a direct NMR method to determine whether the interactions in a Tomonaga-Luttinger liquid (TLL) state of a spin-1 /2 Heisenberg antiferromagnetic ladder are attractive or repulsive. For the strong-leg spin ladder compound (C7H10N )2CuBr4 we find that the isothermal magnetic field dependence of the NMR relaxation rate T1-1(H ) displays a concave curve between the two critical fields bounding the TLL regime. This is in sharp contrast to the convex curve previously reported for a strong-rung ladder, (C5H12N )2CuBr4 . We show that the concavity and the convexity of T1-1(H ), which is a fingerprint of spin fluctuations, directly reflect the attractive and repulsive fermionic interactions in the TLL, respectively. The interaction sign is alternatively determined from an indirect method combining bulk magnetization and specific heat data.

  16. Non-Fermi-Liquid Single Particle Line Shape of the Quasi-One-Dimensional Non-CDW Metal Li{sub 0.9}Mo{sub 6}O{sub 17} : Comparison to the Luttinger Liquid

    SciTech Connect

    Denlinger, J.D.; Gweon, G.; Allen, J.W.; Schlenker, C.; Hsu, L.; Olson, C.G.; Marcus, J.

    1999-03-01

    We report the detailed non-Fermi-liquid (NFL) line shape of the dispersing excitation which defines the Fermi surface for quasi-one-dimensional Li{sub 0.9}Mo {sub 6}O{sub 17} . The properties of Li{sub 0.9}Mo {sub 6}O{sub 17} strongly suggest that the NFL behavior has a purely electronic origin. In relation to the theoretical Luttinger liquid line shape, we identify significant similarities, but also important differences. {copyright} {ital 1999} {ital The American Physical Society}

  17. The Luttinger Sum Rule in Doped Spin Liquids With some speculations about the Pseudogap Phase of the Underdoped Cuprates

    NASA Astrophysics Data System (ADS)

    Rice, T. M.

    2006-02-01

    The Luttinger sum rule is usually considered for Landau Fermi liquids in which the single particle Green's function G(k, 0) changes sign at the the Fermi surface by passing through infinity. However the general proof allows also for a sign change at which G has a zero. A recent analysis by Konik and coworkers considers a model of 2-leg Hubbard ladders weakly coupled by a small long range interladder tunneling. At half-filling a semimetallic state with small Fermi pockets is induced beyond a threshold tunneling strength. The sign changes in G(k, 0) relevent for the Luttinger sum rule now take place at surfaces with both zeros and infinities. The zero surfaces differ from the minimum gap surfaces. The latter are often used in ARPES experiments on underdoped cuprates to obtain an underlying Fermi surface but this procedure leads to problems with the Luttinger sum rule. Some speculations on how the Luttinger sum rule should be applied to the pseudogap phase of the underdoped cuprates are included.

  18. Interplay of topology and interactions in quantum Hall topological insulators: U(1) symmetry, tunable Luttinger liquid, and interaction-induced phase transitions

    NASA Astrophysics Data System (ADS)

    Kharitonov, Maxim; Juergens, Stefan; Trauzettel, Björn

    2016-07-01

    We consider a class of quantum Hall topological insulators: topologically nontrivial states with zero Chern number at finite magnetic field, in which the counterpropagating edge states are protected by a symmetry (spatial or spin) other than time-reversal. HgTe-type heterostructures and graphene are among the relevant systems. We study the effect of electron interactions on the topological properties of the system. We particularly focus on the vicinity of the topological phase transition, marked by the crossing of two Landau levels, where the system is a strongly interacting quantum Hall ferromagnet. We analyze the edge properties using the formalism of the nonlinear σ -model. We establish the symmetry requirement for the topological protection in this interacting system: effective continuous U(1) symmetry with respect to uniaxial isospin rotations must be preserved. If U(1) symmetry is preserved, the topologically nontrivial phase persists; its edge is a helical Luttinger liquid with highly tunable effective interactions. We obtain explicit analytical expressions for the parameters of the Luttinger liquid in the quantum-Hall-ferromagnet regime. However, U(1) symmetry may be broken, either spontaneously or by U(1)-asymmetric interactions. In either case, interaction-induced transitions occur to the respective topologically trivial phases with gapped edge charge excitations.

  19. Long-lived non-equilibrium states in a quantum-Hall Tomonaga-Luttinger liquid

    NASA Astrophysics Data System (ADS)

    Fujisawa, Toshimasa; Washio, Kazuhisa; Nakazawa, Ryo; Hashisaka, Masayuki; Muraki, Koji; Tokura, Yasuhiro

    The existence of long-lived non-equilibrium states without showing thermalization, which has previously been demonstrated in time evolution of ultracold atoms (quantum quench), suggests the possibility of their spatial analogue in transport behavior of interacting electrons in solid-state systems. Here we report long-lived non-equilibrium states in one-dimensional edge channels in the integer quantum Hall regime. For this purpose, non-trivial binary spectrum composed of hot and cold carriers is prepared by an indirect heating scheme using weakly coupled counterpropagating edge channels in an AlGaAs/GaAs heterostructure. Quantum dot spectroscopy clearly reveals that the carriers with the non-trivial binary spectrum propagate over a long distance (5 - 10 um), much longer than the length required for electronic relaxation (about 0.1 um), without thermalization into a trivial Fermi distribution. This observation is consistent with the integrable model of Tomonaga-Luttinger liquid. The long-lived spectrum implies that the system is well described by non-interacting plasmons, which are attractive for carrying information for a long distance. This work was supported by the JSPS 26247051 and 15H05854, and Nanotechnology Platform Program of MEXT.

  20. Fractionalization beyond Luttinger Liquid in the spectroscopy of Lithium Purple Bronze

    NASA Astrophysics Data System (ADS)

    Natalia, Lera; Jose, Alvarez

    We offer an interpretation for the departures of ARPES and STS spectroscopies experiments in quasi-one-dimensional Lithium Purple Bronze (LiPB) from single-band Luttinger Liquid (LL) theory. We base our calculation on a phenomenological description of the published data proposed in the original experiments and consider two bands crossing the Fermi level. We discuss the breakdown of the LL scaling relation η = α - 1 , the separation of the spinon edge and the holon peak, the phenomenological TL fit to the Energy Distribution Curves (EDC) and the survival of power-like density of states down to 4K. We consider non-critical fluctuations in one of the separated modes in which the electron fractionalize, and discuss under which conditions could be related with the upturn in the resistivity at 20-30K. We discuss the possibility of a gap in such separated mode and its role on the robust one-dimensional behavior. The connection with the proposed triplet superconductivity is at T = 1 . 4 K is also studied. We acknowledge financial support from MINECO FIS2012-37549-C05-03.

  1. Pinning quantum phase transition for a Luttinger liquid of strongly interacting bosons.

    PubMed

    Haller, Elmar; Hart, Russell; Mark, Manfred J; Danzl, Johann G; Reichsöllner, Lukas; Gustavsson, Mattias; Dalmonte, Marcello; Pupillo, Guido; Nägerl, Hanns-Christoph

    2010-07-29

    Quantum many-body systems can have phase transitions even at zero temperature; fluctuations arising from Heisenberg's uncertainty principle, as opposed to thermal effects, drive the system from one phase to another. Typically, during the transition the relative strength of two competing terms in the system's Hamiltonian changes across a finite critical value. A well-known example is the Mott-Hubbard quantum phase transition from a superfluid to an insulating phase, which has been observed for weakly interacting bosonic atomic gases. However, for strongly interacting quantum systems confined to lower-dimensional geometry, a novel type of quantum phase transition may be induced and driven by an arbitrarily weak perturbation to the Hamiltonian. Here we observe such an effect--the sine-Gordon quantum phase transition from a superfluid Luttinger liquid to a Mott insulator--in a one-dimensional quantum gas of bosonic caesium atoms with tunable interactions. For sufficiently strong interactions, the transition is induced by adding an arbitrarily weak optical lattice commensurate with the atomic granularity, which leads to immediate pinning of the atoms. We map out the phase diagram and find that our measurements in the strongly interacting regime agree well with a quantum field description based on the exactly solvable sine-Gordon model. We trace the phase boundary all the way to the weakly interacting regime, where we find good agreement with the predictions of the one-dimensional Bose-Hubbard model. Our results open up the experimental study of quantum phase transitions, criticality and transport phenomena beyond Hubbard-type models in the context of ultracold gases. PMID:20671704

  2. Phases of one-dimensional SU(N) cold atomic Fermi gases-From molecular Luttinger liquids to topological phases

    NASA Astrophysics Data System (ADS)

    Capponi, S.; Lecheminant, P.; Totsuka, K.

    2016-04-01

    Alkaline-earth and ytterbium cold atomic gases make it possible to simulate SU(N)-symmetric fermionic systems in a very controlled fashion. Such a high symmetry is expected to give rise to a variety of novel phenomena ranging from molecular Luttinger liquids to (symmetry-protected) topological phases. We review some of the phases that can be stabilized in a one dimensional lattice. The physics of this multi-component Fermi gas turns out to be much richer and more exotic than in the standard SU(2) case. For N > 2, the phase diagram is quite rich already in the case of the single-band model, including a molecular Luttinger liquid (with dominant superfluid instability in the N-particle channel) for incommensurate fillings, as well as various Mott-insulating phases occurring at commensurate fillings. Particular attention will be paid to the cases with additional orbital degree of freedom (which is accessible experimentally either by taking into account two atomic states or by putting atoms in the p-band levels). We introduce two microscopic models which are relevant for these cases and discuss their symmetries and strong coupling limits. More intriguing phase diagrams are then presented including, for instance, symmetry protected topological phases characterized by non-trivial edge states.

  3. Investigation of fermionic pairing on tight binding lattice for low dimensional systems - Fermi liquid vs. Luttinger-Tomonaga liquid

    NASA Astrophysics Data System (ADS)

    Roy Chowdhury, Soumi; Chaudhury, Ranjan

    2015-05-01

    Cooper's original one pair problem in continuum is revisited here corresponding to a lattice of tight binding nature, with an aim to investigate superconductivity in low dimensional systems. An electronic type of boson mediated attraction in a passive Fermi sea-like background is considered for the pairing mechanism with the non-trivial energy dependence of the electronic density of states taken into account in the calculation in a rigorous way. Some of the very important electronic and optical properties in the normal phase of quasi one dimensional organic superconductors are used for the development of the formalism and calculations. The results of our calculations show that a realistic fermionic pair formation is indeed possible with some constraints, without any necessity at all of invoking Luttinger-Tomonaga liquid (LTL) theory. Similarities emerge in the physical properties of the electron pair formed from Cooper's treatment corresponding to continuum and ours, excepting the striking difference appearing in the form of occurrences of a maximum allowed band filling for pairing and of an upper bound of the pairing energy found in our approach.

  4. New Luttinger-Liquid Physics from Photoemission on Li0.9Mo6O17

    SciTech Connect

    Wang, Feng; Alvarez, J V; Mo, S -K; Allen, J W; Gweon, G -H; He, J; Jin, Rongying; Mandrus, David; Hochst, H

    2006-01-01

    Temperature dependent high resolution photoemission spectra of quasi-one-dimensional Li{sub 0.9}Mo{sub 6}O{sub 17} evince a strong renormalization of its Luttinger-liquid density-of-states anomalous exponent. We trace this new effect to interacting charge neutral critical modes that emerge naturally from the two-band nature of the material. Li{sub 0.9}Mo{sub 6}O{sub 17} is shown thereby to be a paradigm material that is capable of revealing new Luttinger physics.

  5. Dimensional phase transition from an array of 1D Luttinger liquids to a 3D Bose-Einstein condensate.

    PubMed

    Vogler, Andreas; Labouvie, Ralf; Barontini, Giovanni; Eggert, Sebastian; Guarrera, Vera; Ott, Herwig

    2014-11-21

    We study the thermodynamic properties of a 2D array of coupled one-dimensional Bose gases. The system is realized with ultracold bosonic atoms loaded in the potential tubes of a two-dimensional optical lattice. For negligible coupling strength, each tube is an independent weakly interacting 1D Bose gas featuring Tomonaga Luttinger liquid behavior. By decreasing the lattice depth, we increase the coupling strength between the 1D gases and allow for the phase transition into a 3D condensate. We extract the phase diagram for such a system and compare our results with theoretical predictions. Because of the high effective mass across the periodic potential and the increased 1D interaction strength, the phase transition is shifted to large positive values of the chemical potential. Our results are prototypical to a variety of low-dimensional systems, where the coupling between the subsystems is realized in a higher spatial dimension such as coupled spin chains in magnetic insulators.

  6. Universal Tomonaga-Luttinger liquid phases in one-dimensional strongly attractive SU(N) fermionic cold atoms

    SciTech Connect

    Guan, X. W.; Lee, J.-Y.; Batchelor, M. T.; Yin, X.-G.; Chen Shu

    2010-08-15

    A simple set of algebraic equations is derived for the exact low-temperature thermodynamics of one-dimensional multicomponent strongly attractive fermionic atoms with enlarged SU(N) spin symmetry and Zeeman splitting. Universal multicomponent Tomonaga-Luttinger liquid (TLL) phases are thus determined. For linear Zeeman splitting, the physics of the gapless phase at low temperatures belongs to the universality class of a two-component asymmetric TLL corresponding to spin-neutral N-atom composites and spin-(N-1)/2 single atoms. The equation of state which we obtained provides a precise description of multicomponent composite fermions and opens up the study of quantum criticality in one-dimensional systems of N-component Fermi gases with population imbalance.

  7. Signatures of Majorana Kramers pairs in superconductor-Luttinger liquid and superconductor-quantum dot-normal lead junctions

    NASA Astrophysics Data System (ADS)

    Kim, Younghyun; Liu, Dong E.; Gaidamauskas, Erikas; Paaske, Jens; Flensberg, Karsten; Lutchyn, Roman M.

    2016-08-01

    Time-reversal invariant topological superconductors are characterized by the presence of Majorana Kramers pairs localized at defects. One of the transport signatures of Majorana Kramers pairs is the quantized differential conductance of 4 e2/h when such a one-dimensional superconductor is coupled to a normal-metal lead. The resonant Andreev reflection, responsible for this phenomenon, can be understood as the boundary condition change for lead electrons at low energies. In this paper, we study the stability of the Andreev reflection fixed point with respect to electron-electron interactions in the Luttinger liquid. We first calculate the phase diagram for the Luttinger liquid-Majorana Kramers pair junction and show that its low-energy properties are determined by Andreev reflection scattering processes in the spin-triplet channel, i.e., the corresponding Andreev boundary conditions are similar to that in a spin-triplet superconductor-normal lead junction. We also study here a quantum dot coupled to a normal lead and a Majorana Kramers pair and investigate the effect of local repulsive interactions leading to an interplay between Kondo and Majorana correlations. Using a combination of renormalization group analysis and slave-boson mean-field theory, we show that the system flows to a new fixed point which is controlled by the Majorana interaction rather than the Kondo coupling. This Majorana fixed point is characterized by correlations between the localized spin and the fermion parity of each spin sector of the topological superconductor. We investigate the stability of the Majorana phase with respect to Gaussian fluctuations.

  8. Time evolution during and after finite-time quantum quenches in Luttinger liquids

    NASA Astrophysics Data System (ADS)

    Chudzinski, Piotr; Schuricht, Dirk

    2016-08-01

    We consider finite-time quantum quenches in the interacting Tomonaga-Luttinger model, for example time-dependent changes of the nearest-neighbor interactions for spinless fermions. We use the exact solutions for specific protocols including the linear and cosine ramps (or, more generally, periodic pumping). We study the dynamics of the total and kinetic energy as well as the Green's functions during as well as after the quench. For the latter we find that the light-cone picture remains applicable; however, the propagating front is delayed as compared to the sudden quench. We extract the universal behavior of the Green's functions and in particular provide analytic, nonperturbative results for the delay applicable to quenches of short to moderate duration but arbitrary time dependency.

  9. Field-induced Tomonaga-Luttinger liquid phase of a two-leg spin-1/2 ladder with strong leg interactions

    SciTech Connect

    Kim, Y. H.; Hotta, C.; Takano, Y.; Tremelling, G.; Turnbull, M. M.; Landee, C.; Kang, H.-J.; Christensen, N. B.; Lefmann, K.; Schmidt, K. P.; Uhrig, G. S.; Broholm, C.

    2010-01-01

    We study the magnetic-field-induced quantum phase transition from a gapped quantum phase that has no magnetic long-range order into a gapless phase in the spin-1/2 ladder compound bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). At temperatures below about 1 K, the specific heat in the gapless phase attains an asymptotic linear temperature dependence, characteristic of a Tomonaga-Luttinger liquid. Inelastic neutron scattering and the specific heat measurements in both phases are in good agreement with theoretical calculations, demonstrating that DIMPY is the first model material for an S=1/2 two-leg spin ladder in the strong-leg regime.

  10. Generalization of Luttinger's Theorem for Fermionic Ladder Systems

    NASA Astrophysics Data System (ADS)

    Gagliardini, P.; Haas, S.; Rice, T. M.; Sigrist, M.

    1998-03-01

    Recently Yamanaka et al.(M. Yamanaka, M. Oshikawa, and I. Affleck, PRL 79), 1110 (1997). adapted the Lieb-Schultz-Mattis theorem to obtain a non-perturbative generalization of Luttinger's theorem for 1-dim. fermionic systems. Their method can be extended to ladder systems. The key quantity which enters in a Hubbard or t-J model is the sum of the electron occupation numbers on a rung. At half-filling, this leads at once to a proof that undoped Heisenberg ladders have gapless excitations when the number of legs is odd. Upon doping, the Fermi wavevectors of individual channels are not conserved under interaction, but their sum is. This result does not require a Fermi surface in each channel and is consistent with the recently proposed assignment of 1 el. per rung to gapped insulating even-parity channels, and 1-δ els. to a Luttinger liquid in the odd-parity channel in a lightly doped 3-leg ladder (δ: hole doping). The crossover to 2 dim. occurs in the limit of a large number of legs, and it is the area enclosed by the Fermi surface which enters, consistent with Luttinger's theorem for the case of Landau Fermi liquids.

  11. Elementary Excitations in Quantum Liquids.

    ERIC Educational Resources Information Center

    Pines, David

    1981-01-01

    Discusses elementary excitations and their role in condensed matter physics, focusing on quantum plasma, helium liquids, and superconductors. Considers research primarily conducted in the 1950s and concludes with a brief survey of some closely related further developments. (Author/JN)

  12. Fermionic approach to junctions of multiple quantum wires attached to Tomonaga-Luttinger liquid leads

    NASA Astrophysics Data System (ADS)

    Shi, Zheng; Affleck, Ian

    2016-07-01

    Junctions of multiple one-dimensional quantum wires of interacting electrons have received considerable theoretical attention as a basic constituent of quantum circuits. While results have been obtained on these models using bosonization and density-matrix renormalization-group (DMRG) methods, another powerful technique is based on direct perturbation theory in the bulk interactions combined with the renormalization group. This technique has so far only been applied to the case in which finite-length interacting wires are attached to noninteracting Fermi liquid leads. We extend this method to cover the case of infinite-length interacting leads, obtaining results on two- and three-lead junctions in good agreement with previous bosonization and DMRG results.

  13. Enhanced NMR Relaxation of Tomonaga-Luttinger Liquids and the Magnitude of the Carbon Hyperfine Coupling in Single-Wall Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Kiss, A.; Pályi, A.; Ihara, Y.; Wzietek, P.; Simon, P.; Alloul, H.; Zólyomi, V.; Koltai, J.; Kürti, J.; Dóra, B.; Simon, F.

    2011-10-01

    Recent transport measurements [Churchill et al. Nature Phys.NPAHAX1745-2473 5, 321 (2009)10.1038/nphys1247] found a surprisingly large, 2-3 orders of magnitude larger than usual C13 hyperfine coupling (HFC) in C13 enriched single-wall carbon nanotubes. We formulate the theory of the nuclear relaxation time in the framework of the Tomonaga-Luttinger liquid theory to enable the determination of the HFC from recent data by Ihara et al. [Europhys. Lett. 90, 17 004 (2010)EULEEJ0295-507510.1209/0295-5075/90/17004]. Though we find that 1/T1 is orders of magnitude enhanced with respect to a Fermi-liquid behavior, the HFC has its usual, small value. Then, we reexamine the theoretical description used to extract the HFC from transport experiments and show that similar features could be obtained with HFC-independent system parameters.

  14. Charge fractionalization in nonchiral Luttinger systems

    NASA Astrophysics Data System (ADS)

    Le Hur, Karyn; Halperin, Bertrand I.; Yacoby, Amir

    2008-12-01

    One-dimensional metals, such as quantum wires or carbon nanotubes, can carry charge in arbitrary units, smaller or larger than a single electron charge. However, according to Luttinger theory, which describes the low-energy excitations of such systems, when a single electron is injected by tunneling into the middle of such a wire, it will tend to break up into separate charge pulses, moving in opposite directions, which carry definite fractions f and (1 - f) of the electron charge, determined by a parameter g that measures the strength of charge interactions in the wire. (The injected electron will also produce a spin excitation, which will travel at a different velocity than the charge excitations.) Observing charge fractionalization physics in an experiment is a challenge in those (nonchiral) low-dimensional systems which are adiabatically coupled to Fermi liquid leads. We theoretically discuss a first important step towards the observation of charge fractionalization in quantum wires based on momentum-resolved tunneling and multi-terminal geometries, and explain the recent experimental results of Steinberg et al. [H. Steinberg, G. Barak, A. Yacoby, L.N. Pfeiffer, K.W. West, B.I. Halperin, K. Le Hur, Nature Physics 4 (2008) 116].

  15. Charge fractionalization in nonchiral Luttinger systems

    SciTech Connect

    Le Hur, Karyn Halperin, Bertrand I.; Yacoby, Amir

    2008-12-15

    One-dimensional metals, such as quantum wires or carbon nanotubes, can carry charge in arbitrary units, smaller or larger than a single electron charge. However, according to Luttinger theory, which describes the low-energy excitations of such systems, when a single electron is injected by tunneling into the middle of such a wire, it will tend to break up into separate charge pulses, moving in opposite directions, which carry definite fractions f and (1-f) of the electron charge, determined by a parameter g that measures the strength of charge interactions in the wire. (The injected electron will also produce a spin excitation, which will travel at a different velocity than the charge excitations.) Observing charge fractionalization physics in an experiment is a challenge in those (nonchiral) low-dimensional systems which are adiabatically coupled to Fermi liquid leads. We theoretically discuss a first important step towards the observation of charge fractionalization in quantum wires based on momentum-resolved tunneling and multi-terminal geometries, and explain the recent experimental results of Steinberg et al. [H. Steinberg, G. Barak, A. Yacoby, L.N. Pfeiffer, K.W. West, B.I. Halperin, K. Le Hur, Nature Physics 4 (2008) 116].

  16. Enhancement of tunneling density of states at a Y junction of spin-1/2 Tomonaga-Luttinger liquid wires

    NASA Astrophysics Data System (ADS)

    Mardanya, Sougata; Agarwal, Amit

    2015-07-01

    We calculate the tunneling density of states (TDOS) in a dissipationless three-wire junction of interacting spin-1/2 electrons, and find an anomalous enhancement of the TDOS in the zero-bias limit, even for repulsive interactions for several bosonic fixed points. This enhancement is physically related to the reflection of holes from the junction for incident electrons, and it occurs only in the vicinity of the junction (x excitations and ω is the bias frequency), crossing over to the bulk value, which is always suppressed at larger distances. The TDOS exponent can be directly probed in an STM experiment by measuring the differential tunneling conductance as a function of either the bias voltage or temperature as done in C. Blumenstein et al., Nat. Phys. 7, 776 (2011), 10.1038/nphys2051.

  17. Liquid storage tanks under vertical excitation

    SciTech Connect

    Philippacopoulos, A.J.

    1985-01-01

    Until recently, the hydrodynamic effects on liquid storage tanks induced by an earthquake excitation were basically treated for the horizontal component of the earthquake. Recent studies, however, showed that the hydrodynamic effects due to the vertical component of an earthquake may be significant. In these studies the tank is assumed to be fixed at the bottom. This paper is concerned with the hydrodynamic behavior of liquid storage tanks induced by vertical earthquake input excitation. First, the fluid-tank system is treated as a fixed-base system and a simple formula is obtained for the coupled fluid-structure natural frequency. Second, additional interaction effects due to the foundation flexibility on the fluid-tank system are investigated. It is concluded that the foundation flexibility may have a significant effect on the hydrodynamic behavior of the liquid storage tanks under a vertical ground shaking.

  18. Tomonaga–Luttinger physics in electronic quantum circuits

    PubMed Central

    Jezouin, S.; Albert, M.; Parmentier, F. D.; Anthore, A.; Gennser, U.; Cavanna, A.; Safi, I.; Pierre, F.

    2013-01-01

    In one-dimensional conductors, interactions result in correlated electronic systems. At low energy, a hallmark signature of the so-called Tomonaga–Luttinger liquids is the universal conductance curve predicted in presence of an impurity. A seemingly different topic is the quantum laws of electricity, when distinct quantum conductors are assembled in a circuit. In particular, the conductances are suppressed at low energy, a phenomenon called dynamical Coulomb blockade. Here we investigate the conductance of mesoscopic circuits constituted by a short single-channel quantum conductor in series with a resistance, and demonstrate a proposed link to Tomonaga–Luttinger physics. We reformulate and establish experimentally a recently derived phenomenological expression for the conductance using a wide range of circuits, including carbon nanotube data obtained elsewhere. By confronting both conductance data and phenomenological expression with the universal Tomonaga–Luttinger conductance curve, we demonstrate experimentally the predicted mapping between dynamical Coulomb blockade and the transport across a Tomonaga–Luttinger liquid with an impurity. PMID:23653214

  19. Tomonaga-Luttinger physics in electronic quantum circuits.

    PubMed

    Jezouin, S; Albert, M; Parmentier, F D; Anthore, A; Gennser, U; Cavanna, A; Safi, I; Pierre, F

    2013-01-01

    In one-dimensional conductors, interactions result in correlated electronic systems. At low energy, a hallmark signature of the so-called Tomonaga-Luttinger liquids is the universal conductance curve predicted in presence of an impurity. A seemingly different topic is the quantum laws of electricity, when distinct quantum conductors are assembled in a circuit. In particular, the conductances are suppressed at low energy, a phenomenon called dynamical Coulomb blockade. Here we investigate the conductance of mesoscopic circuits constituted by a short single-channel quantum conductor in series with a resistance, and demonstrate a proposed link to Tomonaga-Luttinger physics. We reformulate and establish experimentally a recently derived phenomenological expression for the conductance using a wide range of circuits, including carbon nanotube data obtained elsewhere. By confronting both conductance data and phenomenological expression with the universal Tomonaga-Luttinger conductance curve, we demonstrate experimentally the predicted mapping between dynamical Coulomb blockade and the transport across a Tomonaga-Luttinger liquid with an impurity.

  20. Finite-temperature coupled-cluster, many-body perturbation, and restricted and unrestricted Hartree–Fock study on one-dimensional solids: Luttinger liquids, Peierls transitions, and spin- and charge-density waves

    SciTech Connect

    Hermes, Matthew R.; Hirata, So

    2015-09-14

    One-dimensional (1D) solids exhibit a number of striking electronic structures including charge-density wave (CDW) and spin-density wave (SDW). Also, the Peierls theorem states that at zero temperature, a 1D system predicted by simple band theory to be a metal will spontaneously dimerize and open a finite fundamental bandgap, while at higher temperatures, it will assume the equidistant geometry with zero bandgap (a Peierls transition). We computationally study these unique electronic structures and transition in polyyne and all-trans polyacetylene using finite-temperature generalizations of ab initio spin-unrestricted Hartree–Fock (UHF) and spin-restricted coupled-cluster doubles (CCD) theories, extending upon previous work [He et al., J. Chem. Phys. 140, 024702 (2014)] that is based on spin-restricted Hartree–Fock (RHF) and second-order many-body perturbation (MP2) theories. Unlike RHF, UHF can predict SDW as well as CDW and metallic states, and unlike MP2, CCD does not diverge even if the underlying RHF reference wave function is metallic. UHF predicts a gapped SDW state with no dimerization at low temperatures, which gradually becomes metallic as the temperature is raised. CCD, meanwhile, confirms that electron correlation lowers the Peierls transition temperature. Furthermore, we show that the results from all theories for both polymers are subject to a unified interpretation in terms of the UHF solutions to the Hubbard–Peierls model using different values of the electron-electron interaction strength, U/t, in its Hamiltonian. The CCD wave function is shown to encompass the form of the exact solution of the Tomonaga–Luttinger model and is thus expected to describe accurately the electronic structure of Luttinger liquids.

  1. Finite-temperature coupled-cluster, many-body perturbation, and restricted and unrestricted Hartree-Fock study on one-dimensional solids: Luttinger liquids, Peierls transitions, and spin- and charge-density waves.

    PubMed

    Hermes, Matthew R; Hirata, So

    2015-09-14

    One-dimensional (1D) solids exhibit a number of striking electronic structures including charge-density wave (CDW) and spin-density wave (SDW). Also, the Peierls theorem states that at zero temperature, a 1D system predicted by simple band theory to be a metal will spontaneously dimerize and open a finite fundamental bandgap, while at higher temperatures, it will assume the equidistant geometry with zero bandgap (a Peierls transition). We computationally study these unique electronic structures and transition in polyyne and all-trans polyacetylene using finite-temperature generalizations of ab initio spin-unrestricted Hartree-Fock (UHF) and spin-restricted coupled-cluster doubles (CCD) theories, extending upon previous work [He et al., J. Chem. Phys. 140, 024702 (2014)] that is based on spin-restricted Hartree-Fock (RHF) and second-order many-body perturbation (MP2) theories. Unlike RHF, UHF can predict SDW as well as CDW and metallic states, and unlike MP2, CCD does not diverge even if the underlying RHF reference wave function is metallic. UHF predicts a gapped SDW state with no dimerization at low temperatures, which gradually becomes metallic as the temperature is raised. CCD, meanwhile, confirms that electron correlation lowers the Peierls transition temperature. Furthermore, we show that the results from all theories for both polymers are subject to a unified interpretation in terms of the UHF solutions to the Hubbard-Peierls model using different values of the electron-electron interaction strength, U/t, in its Hamiltonian. The CCD wave function is shown to encompass the form of the exact solution of the Tomonaga-Luttinger model and is thus expected to describe accurately the electronic structure of Luttinger liquids. PMID:26374011

  2. Ionization and Excitation in Non-Polar Organic Liquids.

    ERIC Educational Resources Information Center

    Lipsky, Sanford

    1981-01-01

    Reviews recent advances in radiation chemistry concerning the effect of high-energy radiation on organic liquids. Discusses the general nature of excited and ionized states, pathways for decay, the effect of environmental perturbation, the behavior of an electron in a nonpolar liquid, and comparison of photochemical and radiation chemical effects.…

  3. Quantum liquid with deconfined fractional excitations in three dimensions.

    PubMed

    Sikora, Olga; Pollmann, Frank; Shannon, Nic; Penc, Karlo; Fulde, Peter

    2009-12-11

    Excitations which carry "fractional" quantum numbers are known to exist in one dimension in polyacetylene, and in two dimensions, in the fractional quantum Hall effect. Fractional excitations have also been invoked to explain the breakdown of the conventional theory of metals in a wide range of three-dimensional materials. However, the existence of fractional excitations in three dimensions remains highly controversial. In this Letter we report direct numerical evidence for the existence of an extended quantum liquid phase supporting fractional excitations in a concrete, three-dimensional microscopic model-the quantum dimer model on a diamond lattice. We demonstrate explicitly that the energy cost of separating fractional monomer excitations vanishes in this liquid phase, and that its energy spectrum matches that of the Coulomb phase in (3+1)-dimensional quantum electrodynamics.

  4. Elementary excitation and energy landscape in simple liquids

    NASA Astrophysics Data System (ADS)

    Egami, T.

    2014-06-01

    The nature of excitations in liquids has been a subject of debate for a long time. In liquids, phonons are extremely short-lived and marginalized. Instead, recent research results indicate that local topological or configurational excitations (anankeons) are the elementary excitations in high temperature metallic liquids. Local topological excitations are those which locally alter the atomic connectivity network by cutting or forming atomic bonds, and are directly tied to the atomistic origin of viscosity in the liquid. The local potential energy landscape (PEL) of anankeons represents the probability weighted projection of the global PEL to a single atom. The original PEL is an insightful concept, but is highly multi-dimensional and difficult to characterize or even to visualize. A description in terms of the local PEL for anankeons appears to offer a simpler and more effective approach toward this complex problem. At the base of these advances, is the recognition that atomic discreteness and the topology of atomic connectivity are the most crucial features of the structure in liquids, which current nonlinear continuum theories cannot fully capture. These discoveries could open the way to the explanation of various complex phenomena in liquids, such as atomic transport, fragility, and the glass transition, in terms of these excitations.

  5. The liquid to vapor phase transition in excited nuclei

    SciTech Connect

    Elliott, J.B.; Moretto, L.G.; Phair, L.; Wozniak, G.J.; Beaulieu, L.; Breuer, H.; Korteling, R.G.; Kwiatkowski, K.; Lefort, T.; Pienkowski, L.; Ruangma, A.; Viola, V.E.; Yennello, S.J.

    2001-05-08

    For many years it has been speculated that excited nuclei would undergo a liquid to vapor phase transition. For even longer, it has been known that clusterization in a vapor carries direct information on the liquid-vapor equilibrium according to Fisher's droplet model. Now the thermal component of the 8 GeV/c pion + 197 Au multifragmentation data of the ISiS Collaboration is shown to follow the scaling predicted by Fisher's model, thus providing the strongest evidence yet of the liquid to vapor phase transition.

  6. One-dimensional Hubbard-Luttinger model for carbon nanotubes

    NASA Astrophysics Data System (ADS)

    Ishkhanyan, H. A.; Krainov, V. P.

    2015-06-01

    A Hubbard-Luttinger model is developed for qualitative description of one-dimensional motion of interacting Pi-conductivity-electrons in carbon single-wall nanotubes at low temperatures. The low-lying excitations in one-dimensional electron gas are described in terms of interacting bosons. The Bogolyubov transformation allows one to describe the system as an ensemble of non-interacting quasi-bosons. Operators of Fermi excitations and Green functions of fermions are introduced. The electric current is derived as a function of potential difference on the contact between a nanotube and a normal metal. Deviations from Ohm law produced by electron-electron short-range repulsion as well as by the transverse quantization in single-wall nanotubes are discussed. The results are compared with experimental data.

  7. Bosonization of the low energy excitations of Fermi liquids

    SciTech Connect

    Castro Neto, A.H.; Fradkin, E. )

    1994-03-07

    We bosonize the low energy excitations of Fermi liquids in any number of dimensions in the limit of long wavelengths. The bosons are a coherent superposition of electron-hole pairs and are related with the displacements of the Fermi surface in some arbitrary direction. A coherent-state path integral for the bosonized theory is derived and it is shown to represent histories of the shape of the Fermi surface. The Landau theory of Fermi liquids can be obtained from the formalism in the absence of nesting of the Fermi surface and singular interactions. We show that the Landau equation for sound waves is exact in the semiclassical approximation for the bosons.

  8. Edge physics of the quantum spin Hall insulator from a quantum dot excited by optical absorption.

    PubMed

    Vasseur, Romain; Moore, Joel E

    2014-04-11

    The gapless edge modes of the quantum spin Hall insulator form a helical liquid in which the direction of motion along the edge is determined by the spin orientation of the electrons. In order to probe the Luttinger liquid physics of these edge states and their interaction with a magnetic (Kondo) impurity, we consider a setup where the helical liquid is tunnel coupled to a semiconductor quantum dot that is excited by optical absorption, thereby inducing an effective quantum quench of the tunneling. At low energy, the absorption spectrum is dominated by a power-law singularity. The corresponding exponent is directly related to the interaction strength (Luttinger parameter) and can be computed exactly using boundary conformal field theory thanks to the unique nature of the quantum spin Hall edge.

  9. Dissociative ionization of liquid water induced by vibrational overtone excitation

    SciTech Connect

    Natzle, W.C.

    1983-03-01

    Photochemistry of vibrationally activated ground electronic state liquid water to produce H/sup +/ and OH/sup -/ ions has been initiated by pulsed, single-photon excitation of overtone and combination transitions. Transient conductivity measurements were used to determine quantum yields as a function of photon energy, isotopic composition, and temperature. The equilibrium relaxation rate following perturbation by the vibrationally activated reaction was also measured as a function of temperature reaction and isotopic composition. In H/sub 2/O, the quantum yield at 283 +- 1 K varies from 2 x 10/sup -9/ to 4 x 10/sup -5/ for wave numbers between 7605 and 18140 cm/sup -1/. In D/sub 2/O, the dependence of quantum yield on wavelength has the same qualitative shape as for H/sub 2/O, but is shifted to lower quantum yields. The position of a minimum in the quantum yield versus hydrogen mole fraction curve is consistent with a lower quantum yield for excitation of HOD in D/sub 2/O than for excitation of D/sub 2/O. The ionic recombination distance of 5.8 +- 0.5 A is constant within experimental error with temperature in H/sub 2/O and with isotopic composition at 25 +- 1/sup 0/C.

  10. Acoustic excitation of liquid fuel droplets and coaxial jets

    NASA Astrophysics Data System (ADS)

    Rodriguez, Juan Ignacio

    This experimental study focuses on two important problems relevant to acoustic coupling with condensed phase transport processes, with special relevance to liquid rocket engine and airbreathing engine combustion instabilities. The first part of this dissertation describes droplet combustion characteristics of various fuels during exposure to external acoustical perturbations. Methanol, ethanol, a liquid synthetic fuel derived from coal gasification via the Fischer-Tropsch process, and a blend of aviation fuel and the synthetic fuel are used. During acoustic excitation, the droplet is situated at or near a pressure node condition, where the droplet experiences the largest velocity perturbations, and at or near a pressure antinode condition, where the droplet is exposed to minimal velocity fluctuations. For unforced conditions, the values of the droplet burning rate constant K of the different fuels are consistent with data in the literature. The location of the droplet with respect to a pressure node or antinode also has a measurable effect on droplet burning rates, which are different for different fuels and in some cases are as high as 28% above the unforced burning rate value. Estimates of flame extinction due to acoustic forcing for different fuels are also obtained. The second part of this work consists of an experimental study on coaxial jet behavior under non-reactive, cryogenic conditions, with direct applications to flow mixing and unstable behavior characterization in liquid rocket engines. These experiments, conducted with nitrogen, span a range of outer to inner jet momentum flux ratios from 0.013 to 23, and explore subcritical, nearcritical and supercritical pressure conditions, with and without acoustic excitation, for two injector geometries. Acoustic forcing at 3 kHz is utilized to maximize the pressure fluctuations within the chamber acting on the jet, reaching maximum values of 4% of the mean chamber pressure. The effect of the magnitude and phase

  11. On the Kohn-Luttinger conundrum

    SciTech Connect

    Hirata, So; He Xiao

    2013-05-28

    Kohn and Luttinger [Phys. Rev. 118, 41 (1960)] showed that the conventional finite-temperature extension of the second-order many-body perturbation theory had the incorrect zero-temperature limit in metals and, on this basis, argued that the theory was incorrect. We show that this inconsistency arises from the noninclusion of the temperature effect in the energies of the zeroth-order eigenstates of the perturbation theory, which causes not only the Kohn-Luttinger conundrum but also another inconsistency with the zero-temperature many-body perturbation theory, namely, the different rates of divergence of the correlation energy in a homogeneous electron gas (HEG). We propose a renormalized many-body perturbation theory derivable from the finite-temperature extension of the normal-ordered second quantization applied to the denominators of the energy expression, which involves the energies of the zeroth-order states, as well as to the numerators. The renormalized theory is shown to have the correct zero-temperature limit and the same rate of divergence in a HEG as the zero-temperature counterpart, and is, therefore, the correct finite-temperature many-body perturbation theory.

  12. Liquid hydrogen suction dip and slosh wave excitation during draining under normal and reduced gravity environments

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.

    1992-01-01

    The paper discusses the dynamical behavior of vapor ingestion, liquid residual at the incipience of suction dip, slosh wave excitation under normal and reduced gravity and different flow rates during liquid hydrogen draining. Liquid residuals at the incipience of suction dip increase as the values of gravity decrease. Also liquid residuals increase with the draining flow rates. Lower ratio of Bond number and Weber number are unable to excite slosh waves. Lower flow rates and higher gravity excites waves with lower frequencies and higher wave amplitude slosh waves.

  13. Advanced nanoparticle generation and excitation by lasers in liquids.

    PubMed

    Barcikowski, Stephan; Compagnini, Giuseppe

    2013-03-01

    Today, nanoparticles are widely implemented as functional elements onto surfaces, into volumes and as nano-hybrids, resulting for example in bioactive composites and biomolecule conjugates. However, only limited varieties of materials compatible for integration into advanced functional materials are available: nanoparticles synthesized using conventional gas phase processes are often agglomerated into micro powders that are hard to re-disperse into functional matrices. Chemical synthesis methods often lead to impurities of the nanoparticle colloids caused by additives and precursor reaction products. In the last decade, laser ablation and nanoparticle generation in liquids has proven to be a unique and efficient technique to generate, excite, fragment, and conjugate a large variety of nanostructures in a scalable and clean manner. This editorial briefly highlights selected recent advancements and critical aspects in the field of pulsed laser-based nanoparticle generation and manipulation, including exemplary strategies to harvest the unique properties of the laser-generated nanomaterials in the field of biomedicine and catalysis. The presented critical aspects address future assignments such as size control and scale-up.

  14. Instability of interfaces of gas bubbles in liquids under acoustic excitation with dual frequency.

    PubMed

    Zhang, Yuning; Du, Xiaoze; Xian, Haizhen; Wu, Yulin

    2015-03-01

    Instability of interfaces of gas bubbles in liquids under acoustic excitation with dual frequency is theoretically investigated. The critical bubble radii dividing stable and unstable regions of bubbles under dual-frequency acoustic excitation are strongly affected by the amplitudes of dual-frequency acoustic excitation rather than the frequencies of dual-frequency excitation. The limitation of the proposed model is also discussed with demonstrating examples.

  15. Excitation spectra and spin gap of the half-filled Holstein-Hubbard model

    NASA Astrophysics Data System (ADS)

    Hohenadler, Martin; Assaad, Fakher F.

    2013-02-01

    Single- and two-particle excitation spectra of the one-dimensional, half-filled Holstein-Hubbard model are calculated using the continuous-time quantum Monte Carlo method. In the metallic phase, the results are consistent with a Luther-Emery liquid that has gapped spin and single-particle excitations but a gapless charge mode. However, given the initially exponential dependence of the spin gap on the backscattering matrix element, the numerical excitation spectra appear gapless in the weak-coupling regime, and therefore resemble those of a Luttinger liquid. The Mott phase has the expected charge gap and gapless spin excitations. The Peierls state shows a charge, spin, and single-particle gap, a soft phonon mode, backfolded shadow bands, and soliton excitations. Arguments and numerical evidence for the existence of a nonzero spin gap throughout the metallic phase are provided in terms of equal-time spin and charge correlation functions.

  16. Contrasting Behaviours of AC and DC Excited Plasmas in Contact with Liquid

    NASA Astrophysics Data System (ADS)

    Liu, Jingjing; Hu, Xiao

    2013-08-01

    A comparative study of the needle-to-liquid plasma in the continuous mode with DC and AC excitations is detailed in this paper. All plasmas studied here are shown to be glow discharges. This study is based on measurements of several key parameters, including electrical energy, optical emission intensities of active species, rotational and vibrational temperatures, and temperatures of the needle and liquid electrodes. AC plasmas can produce 1.2~5 times higher excited state active species than DC plasmas under the same dissipated power. AC excited liquid plasmas have the highest energy utilization efficiency among the three systems (AC excited plasmas, DC excited plasmas with water anode and DC excited plasmas with water cathode); most of the energy is used to produce useful species rather than to heat the electrodes and plasmas.

  17. Femtosecond solvation dynamics in a neat ionic liquid and ionic liquid microemulsion: excitation wavelength dependence.

    PubMed

    Adhikari, Aniruddha; Sahu, Kalyanasis; Dey, Shantanu; Ghosh, Subhadip; Mandal, Ujjwal; Bhattacharyya, Kankan

    2007-11-01

    Solvation dynamics in a neat ionic liquid, 1-pentyl-3-methyl-imidazolium tetra-flouroborate ([pmim][BF4]) and its microemulsion in Triton X-100 (TX-100)/benzene is studied using femtosecond up-conversion. In both the neat ionic liquid and the microemulsion, the solvation dynamics is found to depend on excitation wavelength (lambda(ex)). The lambda(ex) dependence is attributed to structural heterogeneity in neat ionic liquid (IL) and in IL microemulsion. In neat IL, the heterogeneity arises from clustering of the pentyl groups which are surrounded by a network of cation and anions. Such a nanostructural organization is predicted in many recent simulations and observed recently in an X-ray diffraction study. In an IL microemulsion, the surfactant (TX-100) molecules aggregate in form of a nonpolar peripheral shell around the polar pool of IL. The micro-environment in such an assembly varies drastically over a short distance. The dynamic solvent shift (and average solvation time) in neat IL as well as in IL microemulsions decreases markedly as lambda(ex) increases from 375 to 435 nm. In a [pmim][BF4]/water/TX-100/benzene quaternary microemulsion, the solvation dynamics is slower than that in a microemulsion without water. This is ascribed to the smaller size of the water containing microemulsion. The anisotropy decay in an IL microemulsion is found to be faster than that in neat IL. PMID:17944511

  18. Edge excitations in fractional Chern insulators

    NASA Astrophysics Data System (ADS)

    Luo, Wei-Wei; Chen, Wen-Chao; Wang, Yi-Fei; Gong, Chang-De

    2013-10-01

    Recent theoretical papers have demonstrated the realization of fractional quantum anomalous Hall states (also called fractional Chern insulators) in topological flat band lattice models without an external magnetic field. Such newly proposed lattice systems play a vital role in obtaining a large class of fractional topological phases. Here we report the exact numerical studies of edge excitations for such systems in a disk geometry loaded with hard-core bosons, which will serve as a more viable experimental probe for such topologically ordered states. We find convincing numerical evidence of a series of edge excitations characterized by the chiral Luttinger liquid theory for the bosonic fractional Chern insulators in both the honeycomb disk Haldane model and the kagome-lattice disk model. We further verify these current-carrying chiral edge states by inserting a central flux to test their compressibility.

  19. Slosh wave excitation due to cryogenic liquid reorientation in space-based propulsion system

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.; Lee, C. C.

    1991-01-01

    The objective of the cryogenic fluid management of the spacecraft propulsion system is to develop the technology necessary for acquistion or positioning of liquid and vapor within a tank in reduced gravity to enable liquid outflow or vapor venting. In this study slosh wave excitation induced by the resettling flow field activated by 1.0 Hz medium frequency impulsive reverse gravity acceleration during the course of liquid fluid reorientation with the initiation of geyser for liquid filled levels of 30, 50, and 80 percent have been studied. Characteristics of slosh waves with various frequencies excited are discussed.

  20. Charged-particle interaction with liquids: Ripplon excitations

    NASA Astrophysics Data System (ADS)

    Barberan, Nuria; Garcia-Molina, Rafael; Gras-Marti, Alberto

    1989-07-01

    We calculate the ripplon field contribution to the self-energy of an electron exterior to a liquid for planar and spherical geometries. We compare the full dielectric calculation of the electron-liquid interaction with the simpler alternative method consisting of integrating the electron-atom static-induced-dipolar potential through the whole liquid volume. We obtain good agreement between both methods for a nonpolar liquid such as 4He but differences up to 40% for a polar liquid such as water. We study the conditions under which the ripplon contribution to the self-energy is a perturbation. For an electron moving parallel to a planar liquid surface, we calculate the ripplon contribution to its stopping power. For this dynamical case, we conclude that the alternative method is a good approximation even for polar liquids.

  1. Parametrically excited sectorial oscillation of liquid drops floating in ultrasound.

    PubMed

    Shen, C L; Xie, W J; Wei, B

    2010-04-01

    We report experiments in which the nonaxisymmetric sectorial oscillations of water drops have been excited using acoustic levitation and an active modulation method. The observed stable sectorial oscillations are up to the seventh mode. These oscillations are excited by parametric resonance. The oblate initial shape of the water drops is essential to this kind of excitations. The oscillation frequency increases with mode number but decreases with equatorial radius for each mode number. The data can be well described by a modified Rayleigh equation, without the use of additional parameters. PMID:20481825

  2. Density domains of a photo-excited electron gas on liquid helium

    NASA Astrophysics Data System (ADS)

    Monarkha, Yu. P.

    2016-06-01

    The Coulombic effect on the stability range of the photo-excited electron gas on liquid helium is shown to favor formation of domains of different densities. Domains appear to eliminate or greatly reduce regions with negative conductivity. An analysis of the density domain structure allows explaining remarkable observations reported recently for the photo-excited electron gas.

  3. Liquid hydrogen slosh waves excited by constant reverse gravity acceleration of geyser initiation

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.; Lee, C. C.

    1992-01-01

    The requirement to settle or to position liquid fuel over the outlet end of the spacecraft propellant tank before main engine restart poses a microgravity fluid behavior problem. Resettlement or reorientation of liquid propellant can be accomplished by providing the optimal acceleration to the spacecraft such that the propellant is reoriented over the tank outlet. In this study slosh wave excitation induced by the resettling flowfield during the course of liquid reorientation with the initiation of geyser for liquid-filled levels of 30, 50, 65, 70, and 80 percent have been studied. Characteristics of slosh waves with various frequencies excited are discussed. Slosh wave excitations will affect the fluid stress distribution exerted on the container wall and shift the fluid mass distribution inside the container, which imposes the time-dependent variations in the moment of inertia of the container. This information is important for the spacecraft control during the course of liquid reorientation.

  4. Ionization and excitation in non-polar organic liquids

    SciTech Connect

    Lipsky, S.

    1981-02-01

    Information from 61 different sources is cited in this review article. Since rather comprehensive review articles were published about 10 years ago, this article describes some of the progress made in the field in the last 10 years. Emphasis of this review is on the nature of ionized and electronically excited states but is limited to features having some relevance to radiation chemistry. Some elementary concepts concerning the general nature of excited and ionized states are discussed. (BLM)

  5. A search for manifestation of two types of collective excitations in dynamic structure of a liquid metal: Ab initio study of collective excitations in liquid Na.

    PubMed

    Bryk, Taras; Wax, J-F

    2016-05-21

    Using a combination of ab initio molecular dynamics and several fit models for dynamic structure of liquid metals, we explore an issue of possible manifestation of non-acoustic collective excitations in longitudinal dynamics having liquid Na as a case study. A model with two damped harmonic oscillators (DHOs) in time domain is used for analysis of the density-density time correlation functions. Another similar model with two propagating contributions and three lowest exact sum rules is considered, as well as an extended hydrodynamic model known as thermo-viscoelastic one which permits two types of propagating modes outside the hydrodynamic region to be used for comparison with ab initio obtained time correlation functions and calculations of dispersions of collective excitations. Our results do not support recent suggestions that, even in simple liquid metals, non-hydrodynamics transverse excitations contribute to the longitudinal collective dynamics and can be detected as a DHO-like spectral shape at their transverse frequency. We found that the thermo-viscoelastic dynamic model permits perfect description of the density-density and current-current time correlation functions of the liquid Na in a wide range of wave numbers, which implies that the origin of the non-hydrodynamic collective excitations contributing to longitudinal dynamics can be short-wavelength heat waves. PMID:27208952

  6. Excitation and dynamics of liquid tin micrometer droplet generation

    NASA Astrophysics Data System (ADS)

    Rollinger, B.; Abhari, R. S.

    2016-07-01

    The dynamics of capillary breakup-based droplet generation are studied for an excitation system based on a tunable piezoelectrically actuated oscillating piston, which generates acoustic pressure waves at the dispenser nozzle. First, the non-ideal pressure boundary conditions of droplet breakup are measured using a fast response pressure probe. A structural analysis shows that the axial modes of the excitation system are the main reasons for the resonance peaks in the pressure response. Second, a correlation between the nozzle inlet pressure and the droplet timing jitter is established with the help of experiments and a droplet formation model. With decreasing wave number, the growth rate of the main excitation decreases, while noise contributions with wave numbers with higher growth rates lead to a non-deterministic structure of the droplet train. A highly coherent and monodisperse droplet stream is obtained when the excitation system is tuned to generate high acoustic pressures at the desired operation frequency and when the noise level on the jet is limited. The jet velocity, hence droplet spacing for a set frequency is then adjusted by varying the reservoir pressure, according to the trade-off between lowest wave number and acceptable timing jitter.

  7. Field-dependent molecular ionization and excitation energies: Implications for electrically insulating liquids

    NASA Astrophysics Data System (ADS)

    Davari, N.; Åstrand, P.-O.; Unge, M.; Lundgaard, L. E.; Linhjell, D.

    2014-03-01

    The molecular ionization potential has a relatively strong electric-field dependence as compared to the excitation energies which has implications for electrical insulation since the excited states work as an energy sink emitting light in the UV/VIS region. At some threshold field, all the excited states of the molecule have vanished and the molecule is a two-state system with the ground state and the ionized state, which has been hypothesized as a possible origin of different streamer propagation modes. Constrained density-functional theory is used to calculate the field-dependent ionization potential of different types of molecules relevant for electrically insulating liquids. The low singlet-singlet excitation energies of each molecule have also been calculated using time-dependent density functional theory. It is shown that low-energy singlet-singlet excitation of the type n → π* (lone pair to unoccupied π* orbital) has the ability to survive at higher fields. This type of excitation can for example be found in esters, diketones and many color dyes. For alkanes (as for example n-tridecane and cyclohexane) on the other hand, all the excited states, in particular the σ → σ* excitations vanish in electric fields higher than 10 MV/cm. Further implications for the design of electrically insulating dielectric liquids based on the molecular ionization potential and excitation energies are discussed.

  8. Fractionalized charge excitations in a spin liquid on partially filled pyrochlore lattices.

    PubMed

    Chen, Gang; Kee, Hae-Young; Kim, Yong Baek

    2014-11-01

    We study the Mott transition from a metal to cluster Mott insulators in the 1/4- and 1/8-filled pyrochlore lattice systems [corrected]. It is shown that such Mott transitions can arise due to charge localization in clusters or in tetrahedron units, driven by the nearest-neighbor repulsive interaction. The resulting cluster Mott insulator is a quantum spin liquid with a spinon Fermi surface, but at the same time a novel fractionalized charge liquid with charge excitations carrying half the electron charge. There exist two emergent U(1) gauge fields or "photons" that mediate interactions between spinons and charge excitations, and between fractionalized charge excitations themselves, respectively. In particular, it is suggested that the emergent photons associated with the fractionalized charge excitations can be measured in x-ray scattering experiments. Various other experimental signatures of the exotic cluster Mott insulator are discussed in light of candidate materials with partially filled bands on the pyrochlore lattice.

  9. Spectral function of the Tomonaga-Luttinger model revisited: Power laws and universality

    NASA Astrophysics Data System (ADS)

    Markhof, L.; Meden, V.

    2016-02-01

    We reinvestigate the momentum-resolved single-particle spectral function of the Tomonaga-Luttinger model. In particular, we focus on the role of the momentum dependence of the two-particle interaction V (q ) . Usually, V (q ) is assumed to be a constant and integrals are regularized in the ultraviolet "by hand" employing an ad hoc procedure. As the momentum dependence of the interaction is irrelevant in the renormalization group sense, this does not affect the universal low-energy properties of the model, e.g., exponents of power laws, if all energy scales are sent to zero. If, however, the momentum k is fixed away from the Fermi momentum kF, with |k - kF| setting a nonvanishing energy scale, the details of V (q ) start to matter. We provide strong evidence that any curvature of the two-particle interaction at small transferred momentum q destroys power-law scaling of the momentum-resolved spectral function as a function of energy. Even for |k - kF| much smaller than the momentum-space range of the interaction the spectral line shape depends on the details of V (q ) . The significance of our results for universality in the Luttinger liquid sense, for experiments on quasi-one-dimensional metals, and for recent results on the spectral function of one-dimensional correlated systems taking effects of the curvature of the single-particle dispersion into account ("nonlinear LL phenomenology") is discussed.

  10. Collective excitations in liquid CD4: Neutron scattering and molecular-dynamics simulations

    NASA Astrophysics Data System (ADS)

    Guarini, E.; Bafile, U.; Barocchi, F.; Demmel, F.; Formisano, F.; Sampoli, M.; Venturi, G.

    2005-12-01

    We have investigated the dynamic structure factor S(Q,ω) of liquid CD4 at T = 97.7 K in the wave vector range 2 <= Q/nm-1 <= 15 by means of neutron scattering and molecular-dynamics simulation, in order to study the centre-of-mass collective dynamics. The agreement between the experimental spectra and those simulated using a recent ab initio based intermolecular potential is good, particularly at low Q. Underdamped collective excitations, detected in the whole experimental Q-range, characterize the dynamics of liquid CD4 as markedly different from that of other molecular liquids. Also, the energy and damping of collective excitations in methane are shown to differ considerably, even at the lowest measured Q-values, from those of linearized hydrodynamic modes. An empirical relation, able to reconcile the different wave vector ranges of mode propagation observed in disparate liquids, is investigated.

  11. Excitations in a thin liquid {sup 4}He film from inelastic neutron scattering

    SciTech Connect

    Clements, B.E. |; Godfrin, H.; Krotscheck, E. |; Lauter, H.J.; Leiderer, P.; Passiouk, V. |; Tymczak, C.J.

    1996-05-01

    We perform a thorough analysis of the experimental dynamic structure function measured by inelastic neutron scattering for a low-temperature ({ital T}=0.65 K) four-layer liquid {sup 4}He film. The results are interpreted in light of recent theoretical calculations of the (nonvortex) excitations in thin liquid Bose films. The experimental system consists of four outer liquid layers, adsorbed to two solid inner {sup 4}He layers, which are themselves adsorbed to a graphite substrate. Relatively intense surface (ripplon) and bulklike modes are observed. The analysis of the experimental data gives strong evidence for still other modes and supports the long-standing theoretical predictions of layerlike modes (layer phonons) associated with excitations propagating primarily within the liquid layers comprising the film. The results of the analysis are consistent with the occurrence of level crossings between modes, and the existence of a layer modes for which the theory predicts will propagate in the vicinity of the solid-liquid interface. The theory and experiment agree on the detailed nature of the ripplon; its dispersion at low momenta, its fall off in intensity at intermediate momenta, and the level crossings at high momentum. Similar to experiment, the theory yields an intense mode in the maxon-roton region which is intrepreted as the formation of the bulklike excitation. {copyright} {ital 1996 The American Physical Society.}

  12. Enhanced efficiency in the excitation of higher modes for atomic force microscopy and mechanical sensors operated in liquids

    SciTech Connect

    Penedo, M. Hormeño, S.; Fernández-Martínez, I.; Luna, M.; Briones, F.; Raman, A.

    2014-10-27

    Recent developments in dynamic Atomic Force Microscopy where several eigenmodes are simultaneously excited in liquid media are proving to be an excellent tool in biological studies. Despite its relevance, the search for a reliable, efficient, and strong cantilever excitation method is still in progress. Herein, we present a theoretical modeling and experimental results of different actuation methods compatible with the operation of Atomic Force Microscopy in liquid environments: ideal acoustic, homogeneously distributed force, distributed applied torque (MAC Mode™), photothermal and magnetostrictive excitation. From the analysis of the results, it can be concluded that magnetostriction is the strongest and most efficient technique for higher eigenmode excitation when using soft cantilevers in liquid media.

  13. Inelastic electron and Raman scattering from the collective excitations in quantum wires

    NASA Astrophysics Data System (ADS)

    Kushwaha, Manvir

    2014-03-01

    The nanofabrication technology has taught us that an m-dimensional confining potential imposed upon an n-dimensional electron gas paves the way to a quasi-(n- m)-dimensional electron gas, with m <= n and 1 <= n , m <= 3 . This is the road to the (semiconducting) quasi- n dimensional electron gas systems we have been happily traversing on now for almost two decades. Achieving quasi-one dimensional electron gas (Q-1DEG) led us to some mixed moments in this journey: while the reduced phase space for the scattering led us believe in the route to the faster electron devices, the proximity to the 1D systems left us in the dilemma of describing it as a Fermi liquid or as a Luttinger liquid. No one had ever suspected the potential of the former, but it took quite a while for some to convince the others on the latter. A realistic Q-1DEG system at the low temperatures is best describable as a Fermi liquid rather than as a Luttinger liquid. This has motivated us to employ the Bohm-Pines' full RPA to develop a systematic methodology for the inelastic electron and light scattering from the collective (plasmon) excitations in Q-1DEG [or quantum wires]. We will discuss in detail the results published in AIP Advances 3, 042103 (2013).

  14. Slosh wave and geyser excitations due to liquid hydrogen shut-off during draining in microgravity

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.

    1995-01-01

    The dynamical behavior of liquid hydrogen shut-off during draining, and shut-off at the moment of the incipience of a suction dip have been investigated. It shows that a large amplitude surge is observed for liquid in the container at the moment of liquid hydrogen shut-off in reduced gravity. It also shows that slosh waves accompanied by a strong geyser are developed for surge-related flow fields induced by liquid hydrogen shut-off at the incipience of a suction dip. In the slosh wave excitation, both a lower gravity environment and higher flow rate before the shut-off of liquid draining are resonsible for the initiation of greater amplitude slosh waves. Slosh wave excitation, due to shut-off during liquid hydrogen draining, shift the fluid mass distribution in the container which imposes time-dependent variation in the spacecraft moment of inertia. This provides important information necessary for on-orbit guidance and attitude control of spacecraft.

  15. Superconducting quantum criticality in three-dimensional Luttinger semimetals

    NASA Astrophysics Data System (ADS)

    Boettcher, Igor; Herbut, Igor F.

    2016-05-01

    We study a simple model of three-dimensional fermions close to a quadratic band touching point, built from the celebrated Luttinger single-particle Hamiltonian and an attractive contact interaction between the particles. Such a system displays a quantum critical point between the semimetallic and an s -wave superconducting phase at which the low-energy "Luttinger fermions" are inextricably coupled to the order parameter fluctuations. The quantum critical point is perturbatively accessible near four spatial dimensions, where it features nontrivial scaling with dynamical exponent 1

  16. Bosonic description of a Tomonaga-Luttinger model with impurities

    NASA Astrophysics Data System (ADS)

    Fernández, Victoria; Li, Kang; Naón, Carlos

    1999-04-01

    We extend a recently proposed non-local version of Coleman's equivalence between the Thirring and sine-Gordon models to the case in which the original fermion fields interact with fixed impurities. We explain how our results can be used in the context of one-dimensional strongly correlated systems (the so called Tomonaga-Luttinger model) to study the dependence of the charge-density oscillations on the range of the fermionic interactions.

  17. The Kohn-Luttinger superconductivity in idealized doped graphene

    NASA Astrophysics Data System (ADS)

    Kagan, M. Yu.; Val'kov, V. V.; Mitskan, V. A.; Korovushkin, M. M.

    2014-06-01

    Idealized graphene monolayer is considered neglecting the van der Waals potential of the substrate and the role of the nonmagnetic impurities. The effect of the long-range Coulomb repulsion in an ensemble of Dirac fermions on the formation of the superconducting pairing in a monolayer is studied in the framework of the Kohn-Luttinger mechanism. The electronic structure of graphene is described in the strong coupling Wannier representation on the hexagonal lattice. We use the Shubin-Vonsowsky model which takes into account the intra- and intersite Coulomb repulsions of electrons. The Cooper instability is established by solving the Bethe-Salpeter integral equation, in which the role of the effective interaction is played by the renormalized scattering amplitude. The renormalized amplitude contains the Kohn-Luttinger polarization contributions up to and including the second-order terms in the Coulomb repulsion. We construct the superconductive phase diagram for the idealized graphene monolayer and show that the Kohn-Luttinger renormalizations and the intersite Coulomb repulsion significantly affect the interplay between the superconducting phases with f-, d+id-, and p+ip-wave symmetries of the order parameter.

  18. Liquid draining shut-off induced geyser and slosh wave excitation at suction dip during draining in microgravity

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.

    1992-01-01

    The dynamical behavior of vapor ingestion, liquid residual at the incipience of suction dip, liquid hydrogen shut-off at the incipience of suction dip, and slosh wave excitation under normal and various reduced gravity environments and different flow rates of liquid during draining have been investigated. It shows that the liquid residual at the incipience of suction dip increases as the values of gravity environment decrease from normal gravity to lower reduced gravity, and also that the liquid residual increases as the flow rates of liquid increase during the courses of liquid hydrogen draining. It also shows that slosh waves accompanied by strong geyser are developed for surge-related flowfields at the moment of liquid hydrogen shut-off. Slosh wave excitation, during the liquid hydrogen shut-off, shift the fluid mass distribution in the container which imposes time-dependent variation in spacecraft moment of inertia.

  19. Internal resonance of nonlinear sloshing in rectangular liquid tanks subjected to obliquely horizontal excitation

    NASA Astrophysics Data System (ADS)

    Ikeda, Takashi; Harata, Yuji; Osasa, Takefumi

    2016-01-01

    Nonlinear sloshing in rectangular tanks subjected to obliquely horizontal, harmonic excitation is investigated when the internal resonance condition 1:1 is satisfied between the natural frequencies of predominate modes (1, 0) and (0, 2). Galerkin's method is employed to derive the nonlinear modal equations of motion for sloshing, considering nine sloshing modes. Then, van der Pol's method is applied in order to obtain the expressions of the frequency response curves for amplitudes and phase angles of the predominate modes. The frequency response curves are calculated and reveal that (0, 2) mode may occur even though it is not directly excited because it is nonlinearly coupled with (1, 0) mode due to the autoparametric terms. In the numerical simulations, it is found that planar motions of (1, 0) mode, clockwise and counter-clockwise swirl motions, and translational motions may appear. Furthermore, Hopf bifurcation occurs, and amplitude modulated motions (AMMs), including chaotic motions, may appear depending on the value of the excitation frequency. Three-dimensional distribution charts of the maximum liquid surface elevation are calculated to show the risk of liquid overspill. The influence of the difference between the horizontal excitation direction and the tank side on the frequency response curves is also examined. Bifurcation sets are calculated to clarify this influence. Experimental data confirmed the validity of the theoretical results.

  20. Fractional Wigner Crystal in the Helical Luttinger Liquid.

    PubMed

    Traverso Ziani, N; Crépin, F; Trauzettel, B

    2015-11-13

    The properties of the strongly interacting edge states of two dimensional topological insulators in the presence of two-particle backscattering are investigated. We find an anomalous behavior of the density-density correlation functions, which show oscillations that are neither of Friedel nor of Wigner type: they, instead, represent a Wigner crystal of fermions of fractional charge e/2, with e the electron charge. By studying the Fermi operator, we demonstrate that the state characterized by such fractional oscillations still bears the signatures of spin-momentum locking. Finally, we compare the spin-spin correlation functions and the density-density correlation functions to argue that the fractional Wigner crystal is characterized by a nontrivial spin texture.

  1. Wentzel-Bardeen singularity in coupled Luttinger liquids: Transport properties

    SciTech Connect

    Martin, T.

    1994-08-26

    The recent progress on 1 D interacting electrons systems and their applications to study the transport properties of quasi one dimensional wires is reviewed. We focus on strongly correlated elections coupled to low energy acoustic phonons in one dimension. The exponents of various response functions are calculated, and their striking sensitivity to the Wentzel-Bardeen singularity is discussed. For the Hubbard model coupled to phonons the equivalent of a phase diagram is established. By increasing the filling factor towards half filling the WB singularity is approached. This in turn suppresses antiferromagnetic fluctuations and drives the system towards the superconducting regime, via a new intermediate (metallic) phase. The implications of this phenomenon on the transport properties of an ideal wire as well as the properties of a wire with weak or strong scattering are analyzed in a perturbative renormalization group calculation. This allows to recover the three regimes predicted from the divergence criteria of the response functions.

  2. Tomonaga-Luttinger liquid theory for metallic fullurene polymers

    NASA Astrophysics Data System (ADS)

    Yoshioka, Hideo; Shima, Hiroyuki; Noda, Yusuke; Ono, Shota; Ohno, Kaoru

    2016-04-01

    We investigate the low energy behavior of local density of states in metallic C60 polymers theoretically. The multichannel bosonization method is applied to electronic band structures evaluated from first-principles calculation, by which the effects of electronic correlation and nanoscale corrugation in the atomic configuration are fully taken into account. We obtain a closed-form expression for the power-law anomalies in the local density of states, which successfully describes the experimental observation on the C60 polymers in a quantitative manner. An important implication from the closed-form solution is the existence of an experimentally unobserved crossover at nearly a hundred milli-electron volts, beyond which the power-law exponent of the C60 polymers should change significantly.

  3. Red and blue shift of liquid water's excited states: A many body perturbation study

    NASA Astrophysics Data System (ADS)

    Ziaei, Vafa; Bredow, Thomas

    2016-08-01

    In the present paper, accurate optical absorption spectrum of liquid H2O is calculated in the energy range of 5-20 eV to probe the nature of water's excited states by means of many body perturbation approach. Main features of recent inelastic X-ray measurements are well reproduced, such as a bound excitonic peak at 7.9 eV with a shoulder at 9.4 eV as well as the absorption maximum at 13.9 eV, followed by a broad shoulder at 18.4 eV. The spectrum is dominated by excitonic effects impacting the structures of the spectrum at low and higher energy regimes mixed by single particle effects at high energies. The exciton distribution of the low-energy states, in particular of S1, is highly anisotropic and localized mostly on one water molecule. The S1 state is essentially a HOCO-LUCO (highest occupied crystal orbital - lowest unoccupied crystal orbital) transition and of intra-molecular type, showing a localized valence character. Once the excitation energy is increased, a significant change in the character of the electronically excited states occurs, characterized through emergence of multiple quasi-particle peaks at 7.9 eV in the quasi-particle (QP) transition profile and in the occurring delocalized exciton density distribution, spread over many more water molecules. The exciton delocalization following a change of the character of excited states at around 7.9 eV causes the blue shift of the first absorption band with respect to water monomer S1. However, due to reduction of the electronic band gap from gas to liquid phase, following enhanced screening upon condensation, the localized S1 state of liquid water is red-shifted with respect to S1 state of water monomer. For higher excitations, near vertical ionization energy (11 eV), quasi-free electrons emerge, in agreement with the conduction band electron picture. Furthermore, the occurring red and blue shift of the excited states are independent of the coupling of resonant and anti-resonant contributions to the

  4. Emergence of nontrivial magnetic excitations in a spin-liquid state of kagomé volborthite.

    PubMed

    Watanabe, Daiki; Sugii, Kaori; Shimozawa, Masaaki; Suzuki, Yoshitaka; Yajima, Takeshi; Ishikawa, Hajime; Hiroi, Zenji; Shibauchi, Takasada; Matsuda, Yuji; Yamashita, Minoru

    2016-08-01

    When quantum fluctuations destroy underlying long-range ordered states, novel quantum states emerge. Spin-liquid (SL) states of frustrated quantum antiferromagnets, in which highly correlated spins fluctuate down to very low temperatures, are prominent examples of such quantum states. SL states often exhibit exotic physical properties, but the precise nature of the elementary excitations behind such phenomena remains entirely elusive. Here, we use thermal Hall measurements that can capture the unexplored property of the elementary excitations in SL states, and report the observation of anomalous excitations that may unveil the unique features of the SL state. Our principal finding is a negative thermal Hall conductivity [Formula: see text] which the charge-neutral spin excitations in a gapless SL state of the 2D kagomé insulator volborthite Cu3V2O7(OH)2[Formula: see text]2H2O exhibit, in much the same way in which charged electrons show the conventional electric Hall effect. We find that [Formula: see text] is absent in the high-temperature paramagnetic state and develops upon entering the SL state in accordance with the growth of the short-range spin correlations, demonstrating that [Formula: see text] is a key signature of the elementary excitation formed in the SL state. These results suggest the emergence of nontrivial elementary excitations in the gapless SL state which feel the presence of fictitious magnetic flux, whose effective Lorentz force is found to be less than 1/100 of the force experienced by free electrons. PMID:27439874

  5. Semiclassical Time Evolution of the Holes from Luttinger Hamiltonian

    SciTech Connect

    Jiang, Z.F.; Li, R.D.; Zhang, Shou-Cheng; Liu1, W.M.; /Beijing, Inst. Phys.

    2010-02-15

    We study the semi-classical motion of holes by exact numerical solution of the Luttinger model. The trajectories obtained for the heavy and light holes agree well with the higher order corrections to the abelian and the non-abelian adiabatic theories in Ref. [1] [S. Murakami et al., Science 301, 1378 (2003)], respectively. It is found that the hole trajectories contain rapid oscillations reminiscent of the 'Zitterbewegung' of relativistic electrons. We also comment on the non-conservation of helicity of the light holes.

  6. Steady States and Universal Conductance in a Quenched Luttinger Model

    NASA Astrophysics Data System (ADS)

    Langmann, Edwin; Lebowitz, Joel L.; Mastropietro, Vieri; Moosavi, Per

    2016-05-01

    We obtain exact analytical results for the evolution of a 1+1-dimensional Luttinger model prepared in a domain wall initial state, i.e., a state with different densities on its left and right sides. Such an initial state is modeled as the ground state of a translation invariant Luttinger Hamiltonian {H_{λ}} with short range non-local interaction and different chemical potentials to the left and right of the origin. The system evolves for time t > 0 via a Hamiltonian {H_{λ'}} which differs from {H_{λ}} by the strength of the interaction. Asymptotically in time, as {t to &infty}; , after taking the thermodynamic limit, the system approaches a translation invariant steady state. This final steady state carries a current I and has an effective chemical potential difference {μ+ - μ-} between right- (+) and left- (-) moving fermions obtained from the two-point correlation function. Both I and {μ+ - μ-} depend on {λ} and {λ'} . Only for the case {λ = λ' = 0} does {μ+ - μ-} equal the difference in the initial left and right chemical potentials. Nevertheless, the Landauer conductance for the final state, {G = I/(μ+ - μ-)} , has a universal value equal to the conductance quantum {e^2/h} for the spinless case.

  7. Development of High-Throughput Liquid Treatment System using Slot Antenna Excited Microwave Plasma

    NASA Astrophysics Data System (ADS)

    Takitou, Sho; Ito, Michiko; Takashima, Seigou; Nomura, Norio; Kitagawa, Tominori; Toyoda, Hirotaka

    2015-09-01

    Recently, much attention has been given to plasma production under liquid and its industrial applications as well as investigation of chemical reactions as a result of plasma-liquid interactions. In various kinds of plasma production techniques, we have proposed pulsed microwave excited plasma using slot antenna, where damage to the slot electrode can be minimized and plasma volume can be increased. Furthermore, we have proposed an in-line microwave plasma system where plasma is efficiently produced under reduced pressures using Venturi effect, and have demonstrated enhancement of organic decomposition efficiency. For practical use of the plasma liquid treatment, however, cost-effective and more efficient treatment system with high treatment capability is required. In this study, we propose further enhancement of the treatment speed by designing four-parallel-type liquid treatment device where four discharges for the treatment are performed using one microwave power source. Decomposition speed of newly-developed plasma system is investigated. Not only high decomposition rate but also enhanced energy efficiency is realized.

  8. Multiphoton Ionization and Two-Photon Excitation of Aromatic Molecules in Liquids

    NASA Astrophysics Data System (ADS)

    Faidas, Homer

    1985-12-01

    The two-photon excitation of benzene and toluene in a number of different nonpolar liquids (n-pentane, tetramethylsilane, perfluoro-n-hexane, perfluoromethylcyclohexane, and perfluorodimethylcyclobutane) was studied over the 360-560 nm laser excitation wavelength range. The effect of the solvent on the upper excited states was investigated and a peak, observed in the two -photon excitation spectra of benzene, was assigned to the (3s)('1)E(,1g) Rydberg state based on the unusual solvent dependence of its relative intensity and spectral shift. Polarization studies and signal vs. laser intensity measurements were also carried out. Virbrational analyses of the entire range of the ('1)B(,2u) state of benzene and of the ('1)B(,2) state of toluene, including the hot bands, were performed based on the spectra measured in perfluoro-n-hexane. The O-O transitions of these states in perfluoro-n-hexane and n -pentane were observed at 38050 cm('-1) and 37853 cm('-1) for benzene and at 37411 cm('-1) and 37220 cm('-1) for toluene, respectively. The two-photon excitation spectrum of fluoranthene in a solution of n-pentane over the 420-860 nm laser excitation range was also measured. The O-O transition of the first singlet state was observed at 24800 cm('-1), resolving thus the ambiguity about the exact position of that state. The multiphoton ionization of benzene in dilute solutions of n-pentane and tetramethylsilane was also studied, over the 360-570 nm laser excitation range. Polarization studies and signal vs. laser intensity measurements were performed and the dependence of the spectral features and of the polarization ratio on the laser intensity was studied. The multiphoton ionization mechanism, the location of the ionization threshold of benzene in n-pentane and in tetramethylsilane and the effect of the medium on the ionization threshold are discussed. A particular ionization behavior was observed in a wavelength region corresponding to the channel 3 relaxation which

  9. Emergence of nontrivial magnetic excitations in a spin-liquid state of kagomé volborthite

    NASA Astrophysics Data System (ADS)

    Watanabe, Daiki; Sugii, Kaori; Shimozawa, Masaaki; Suzuki, Yoshitaka; Yajima, Takeshi; Ishikawa, Hajime; Hiroi, Zenji; Shibauchi, Takasada; Matsuda, Yuji; Yamashita, Minoru

    2016-08-01

    When quantum fluctuations destroy underlying long-range ordered states, novel quantum states emerge. Spin-liquid (SL) states of frustrated quantum antiferromagnets, in which highly correlated spins fluctuate down to very low temperatures, are prominent examples of such quantum states. SL states often exhibit exotic physical properties, but the precise nature of the elementary excitations behind such phenomena remains entirely elusive. Here, we use thermal Hall measurements that can capture the unexplored property of the elementary excitations in SL states, and report the observation of anomalous excitations that may unveil the unique features of the SL state. Our principal finding is a negative thermal Hall conductivity κxyκxy which the charge-neutral spin excitations in a gapless SL state of the 2D kagomé insulator volborthite Cu3V2O7(OH)2ṡ2H2O exhibit, in much the same way in which charged electrons show the conventional electric Hall effect. We find that κxyκxy is absent in the high-temperature paramagnetic state and develops upon entering the SL state in accordance with the growth of the short-range spin correlations, demonstrating that κxyκxy is a key signature of the elementary excitation formed in the SL state. These results suggest the emergence of nontrivial elementary excitations in the gapless SL state which feel the presence of fictitious magnetic flux, whose effective Lorentz force is found to be less than 1/100 of the force

  10. Cholesteric liquid crystal laser in a dielectric mirror cavity upon band-edge excitation

    NASA Astrophysics Data System (ADS)

    Matsuhisa, Yuko; Huang, Yuhua; Zhou, Ying; Wu, Shin-Tson; Takao, Yuuki; Fujii, Akihiko; Ozaki, Masanori

    2007-01-01

    Low threshold laser action of dye-doped cholesteric liquid crystals (CLCs) is demonstrated using an input circularly polarized light whose handedness is the same as the cholesteric helix of the sample at the high-energy band edge of the reflection band. The mechanism originates from the dramatic increase of the photon density of state at the band edges. We also demonstrate an enhanced laser action of a CLC in a dielectric multilayer cavity. In such a device configuration, the band-edge excitation at high-energy band edge improves the lasing performance not only for the same handedness circularly polarized pump beam as the cholesteric helix but also for the opposite one. It stems from the polarization independence of the dielectric multilayers.

  11. Thermally excited fluid flow in a microsized liquid crystal channel with a free surface

    NASA Astrophysics Data System (ADS)

    Zakharov, A. V.; Vakulenko, A. A.

    2015-06-01

    The temperature-induced reorientation dynamics in microsized liquid crystal (LC) channel with a free LC/vacuum interface has been investigated theoretically based on the hydrodynamic theory including the director motion, the thermally excited fluid flow v, and the temperature T redistribution, produced by induced heating in the interior of the LC sample. Analysis of the numerical results shows that due to interaction between ∇T and the gradient of the director field ∇ n ˆ in the LC channel bounded by the free LC/vacuum interface, a thermally excited vortical fluid flow is maintained in the vicinity of the heat source. Calculations also show that in the case of the fast heating, the LC sample settles down to three-vortical flow regime, whereas in the case of the slow heating, the LC material settles down to bi-vortical flow regime. As for nematogenic material, we have considered the LC channel to be occupied by 4-n-pentyl-4'-cyanobiphenyl and investigated the effect of both ∇ n ˆ and ∇T on the magnitude and direction of v, as well as on the height of the LC film on the solid surface, for a number of heating and hydrodynamic regimes.

  12. Investigating the role of vibrational excitation in simulating charged-particle tracks in liquid pyrimidine

    NASA Astrophysics Data System (ADS)

    Brunger, Michael J.; Ratnavelu, Kuru; Buckman, Stephen J.; Jones, Darryl B.; Muñoz, Antonio; Blanco, Francisco; García, Gustavo

    2016-03-01

    We report on our results of a study into the sensitivity of charged-particle (electron) track simulations in liquid pyrimidine, to the vibrational cross sections and vibrational energy loss distribution function employed in those simulations. We achieve this by repeating the earlier investigation of Fuss et al. [J. Appl. Phys. 117, 214701 (2015)], but now incorporating more accurate data for the vibrational integral cross sections and the energy loss distribution function that have recently become available. We find that while changes in absorbed dose or particle range are quite minor, due to the energy transferred via vibrational excitations being low in comparison to that for other processes such as ionisation, at the very end of the tracks, where non-ionizing interactions dominate, the significantly large numbers of vibrational excitation processes increases the electrons' ability to induce other effects (e.g. sample heating, bond breaking and radical formation) that might cause damage. Contribution to the Topical Issue "Advances in Positron and Electron Scattering", edited by Paulo Limao-Vieira, Gustavo Garcia, E. Krishnakumar, James Sullivan, Hajime Tanuma and Zoran Petrovic.

  13. Ultrafast spectroscopy of electron transfer dynamics in liquids; excitation transfer studies of phase transitions

    NASA Astrophysics Data System (ADS)

    Goun, Alexei A.

    tetradecyltrimethylammonium bromide (TTAB). It was found that the effective coupling is reduced compared to donor/acceptor pairs dissolved in simple liquids. In the 2nd half of thesis we have addressed the question of the dynamics of phase transitions. We have demonstrated the ability to use the fluorescent excitation-transfer technique to study the demixing of liquids specifically, kinetics of demixing water and 2,6-dimethylpyridine. These two liquids possess a low critical temperature point, which allowed us to use a temperature jump from a laser pulse to initiate the process of phase separation. It was found that Coumarin480 laser dye and HPTS (8-Hydroxypyrene-1,3,6-trisulfonic acid) fluorescent dye have significantly different solubilities in the components of the mixture. These dyes undergo excitation transfer from Coumarin480 to HPTS in the uniform state, but not in the phase-separated state. A system with a temperature jump pump and an excitation transfer probe measured the time scale of the initial step of the phase separation.

  14. Topological Influence of Lyotropic Liquid Crystalline Systems on Excited-State Proton Transfer Dynamics.

    PubMed

    Roy, Bibhisan; Satpathi, Sagar; Hazra, Partha

    2016-03-29

    In the present work, we have investigated the excited-state proton transfer (ESPT) dynamics inside lipid-based reverse hexagonal (HII), gyroid Ia3d, and diamond Pn3m LLC phases. Polarized light microscopy (PLM) and small-angle X-ray scattering (SAXS) techniques have been employed for the characterization of LLC systems. Time-resolved fluorescence results reveal the retarded ESPT dynamics inside liquid crystalline systems compared to bulk water, and it follows the order HII < Ia3d < Pn3m < H2O. The slower solvation, hampered "Grotthuss" proton transfer process, and most importantly, topological influence, of the LLC systems are believed to be mainly responsible for the slower and different extent of ESPT dynamics. Interestingly, recombination dynamics is found to be faster with respect to bulk water and it follows the order H2O < Pn3m < Ia3d < HII. Faster recombination dynamics arises due to lower dielectric constant and different channel diameters of these LLC systems. However, the dissociation dynamics is found to be slower than bulk water and it follows the order HII < Ia3d < Pn3m < H2O. Differences in critical packing parameter of LLC systems are believed to be the governing factors for the slower dissociation dynamics in these liquid crystalline systems.

  15. Large temperature renormalization of anomalous Luttinger exponent in Li0.9Mo6O17

    NASA Astrophysics Data System (ADS)

    Wang, Feng; Mo, S.-K.; Allen, J. W.; Alvarez, J. V.; Gweon, G.-H.; He, J.; Jin, R.; Mandrus, R.; Höchst, H.

    2006-03-01

    Li0.9Mo6O17 is unique as a quasi-1 dimensional metal for which both photoemission spectroscopy (PES) [1] and tunneling [2] find Luttinger liquid (LL) power law behaviors in spectra near the Fermi energy EF, albeit with differing values of the anomalous exponent α, 0.9 at temperature 300K and 0.6 below 50K, respectively. New T-dependent PES spectra from T = 300K down to 15K can be well fit by finite-T LL theory, with α varying continuously from 0.9 to 0.6, showing consistency of PES and tunneling. We find that its incommensurate Fermi wavevector would preclude such a large renormalization of α with T for Li0.9Mo6O17 were it not for interband dynamics and residual interaction scattering that can occur only because there are two (nearly degenerate) bands crossing EF. We also discuss implications of the theory for further experiments. [1] G.-H. Gweon et al, Phys. Rev. B 68, 195117 (2003). [2] J. Hager et al, Phys. Rev. Lett. 95, 186402 (2005).

  16. Liquid sloshing in partly-filled laterally-excited circular tanks equipped with baffles

    NASA Astrophysics Data System (ADS)

    Hasheminejad, Seyyed M.; Mohammadi, M. M.; Jarrahi, Miad

    2014-01-01

    Linear potential theory in conjunction with the conformal mapping technique are employed to develop rigorous mathematical models for two-dimensional transient sloshing in non-deformable baffled horizontal circular cylindrical vessels, filled with inviscid incompressible fluids to arbitrary depths, and subjected to arbitrary time-dependent lateral accelerations. Three common baffle configurations are considered, namely, a pair of free surface-touching horizontal side baffles, and a central surface-piercing or bottom-mounted vertical baffle of arbitrary extension. The first few normalized antisymmetric/symmetric sloshing frequencies of the partially-filled tanks are tabulated for selected baffle extension and fill depth ratios. Also, the effects of liquid fill depth or baffle length parameter on the impulsive, total and modal convective mass ratios are examined. A ramp-step function is used to replicate the lateral acceleration excitation encountered in an idealized turning maneuver. Durbin's numerical Laplace transform inversion scheme was applied to solve the resulting truncated linear sets of ordinary differential equations in the time-domain. The effects of excitation input time, fill level, and baffle configuration/extension on the force and moment amplification factors are illustrated through appropriate design charts. Furthermore, the transient hydrodynamic responses to a real seismic event are calculated and the effectiveness of baffle configuration/length on suppression of the induced destabilizing lateral forces are examined. Limiting cases are considered and rigorous verifications are made by comparison with the available data as well as with the numerical simulations performed by using a commercial CFD software package.

  17. Inelastic electron and Raman scattering from the collective excitations in quantum wires: Zero magnetic field

    NASA Astrophysics Data System (ADS)

    Kushwaha, Manvir S.

    2013-04-01

    The nanofabrication technology has taught us that an m-dimensional confining potential imposed upon an n-dimensional electron gas paves the way to a quasi-(n-m)-dimensional electron gas, with m ⩽ n and 1 ⩽ n, m ⩽ 3. This is the road to the (semiconducting) quasi-n dimensional electron gas systems we have been happily traversing on now for almost two decades. Achieving quasi-one dimensional electron gas (Q-1DEG) [or quantum wire(s) for more practical purposes] led us to some mixed moments in this journey: while the reduced phase space for the scattering led us believe in the route to the faster electron devices, the proximity to the 1D systems left us in the dilemma of describing it as a Fermi liquid or as a Luttinger liquid. No one had ever suspected the potential of the former, but it took quite a while for some to convince the others on the latter. A realistic Q-1DEG system at the low temperatures is best describable as a Fermi liquid rather than as a Luttinger liquid. In the language of condensed matter physics, a critical scrutiny of Q-1DEG systems has provided us with a host of exotic (electronic, optical, and transport) phenomena unseen in their higher- or lower-dimensional counterparts. This has motivated us to undertake a systematic investigation of the inelastic electron scattering (IES) and the inelastic light scattering (ILS) from the elementary electronic excitations in quantum wires. We begin with the Kubo's correlation functions to derive the generalized dielectric function, the inverse dielectric function, and the Dyson equation for the dynamic screened potential in the framework of Bohm-Pines' random-phase approximation. These fundamental tools then lead us to develop methodically the theory of IES and ILS for the Q-1DEG systems. As an application of the general formal results, which know no bounds regarding the subband occupancy, we compute the density of states, the Fermi energy, the full excitation spectrum [comprised of intrasubband and

  18. Photothermal excitation and laser Doppler velocimetry of higher cantilever vibration modes for dynamic atomic force microscopy in liquid

    SciTech Connect

    Nishida, Shuhei; Kobayashi, Dai; Sakurada, Takeo; Nakazawa, Tomonori; Hoshi, Yasuo; Kawakatsu, Hideki

    2008-12-15

    The authors present an optically based method combining photothermal excitation and laser Doppler velocimetry of higher cantilever vibration modes for dynamic atomic force microscopy in liquid. The frequency spectrum of a silicon cantilever measured in water over frequencies ranging up to 10 MHz shows that the method allows us to excite and detect higher modes, from fundamental to fifth flexural, without enhancing spurious resonances. By reducing the tip oscillation amplitude using higher modes, the average tip-sample force gradient due to chemical bonds is effectively increased to achieve high-spatial-resolution imaging in liquid. The method's performance is demonstrated by atomic resolution imaging of a mica surface in water obtained using the second flexural mode with a small tip amplitude of 99 pm; individual atoms on the surface with small height differences of up to 60 pm are clearly resolved.

  19. Ultrafast FRET in a room temperature ionic liquid microemulsion: a femtosecond excitation wavelength dependence study.

    PubMed

    Adhikari, Aniruddha; Das, Dibyendu Kumar; Sasmal, Dibyendu Kumar; Bhattacharyya, Kankan

    2009-04-23

    Fluorescence resonance energy transfer (FRET) from coumarin 480 (C480) to rhodamine 6G (R6G) is studied in a room temperature ionic liquid (RTIL) microemulsion by picosecond and femtosecond emission spectroscopy. The microemulsion is comprised of the RTIL 1-pentyl-3-methylimidazolium tetraflouroborate, [pmim][BF4], in TX-100/ benzene. We have studied the microemulsion with and without water. The time constants of FRET were obtained from the risetime of the acceptor (R6G) emission. In the RTIL microemulsion, FRET occurs on multiple time scales: 1, 250, and 3900 ps. In water containing RTIL microemulsion, the rise components are 1.5, 250, and 3900 ps. The 1 and 1.5 ps components are assigned to FRET at a close contact of donor and acceptor (RDA approximately 12 A). This occurs within the highly polar (RTIL/water) pool of the microemulsion. With increase in the excitation wavelength (lambdaex) from 375 to 435 nm, the relative contribution of the ultrafast component of FRET (1 ps) increases from 4% to 100% in the RTIL microemulsion and 12% to 100% in the water containing RTIL microemulsion. It is suggested that at lambdaex = 435 nm, mainly the highly polar RTIL pool is probed where FRET is very fast due to the close proximity of the donor and the acceptor. The very long 3900 ps (RDA approximately 45 A) component may arise from FRET from a donor in the outer periphery of the microemulsion to an acceptor in the polar RTIL pool. The 250 ps component (RDA approximately 29 A) is assigned to FRET from a donor inside the surfactant chains. PMID:19127996

  20. Contribution of tuned liquid column gas dampers to the performance of offshore wind turbines under wind, wave, and seismic excitations

    NASA Astrophysics Data System (ADS)

    Bargi, Khosrow; Dezvareh, Reza; Mousavi, Seyed Amin

    2016-09-01

    The main intention of the present study is to reduce wind, wave, and seismic induced vibrations of jackettype offshore wind turbines (JOWTs) through a newly developed vibration absorber, called tuned liquid column gas damper (TLCGD). Using a Simulink-based model, an analytical model is developed to simulate global behavior of JOWTs under different dynamic excitations. The study is followed by a parametric study to explore efficiency of the TLCGD in terms of nacelle acceleration reduction under wind, wave, and earthquake loads. Study results indicate that optimum frequency of the TLCGD is rather insensitive to excitation type. In addition, while the gain in vibration control from TLCGDs with higher mass ratios is generally more pronounced, heavy TLCGDs are more sensitive to their tuned frequency such that ill-regulated TLCGD with high mass ratio can lead to destructive results. It is revealed that a well regulated TLCGD has noticeable contribution to the dynamic response of the JOWT under any excitation.

  1. An atmospheric air gas-liquid diffuse discharge excited by bipolar nanosecond pulse in quartz container used for water sterilization

    NASA Astrophysics Data System (ADS)

    Wang, Sen; Yang, De-Zheng; Wang, Wen-Chun; Zhang, Shuai; Liu, Zhi-Jie; Tang, Kai; Song, Ying

    2013-12-01

    In this Letter, we report that the air gas-liquid diffuse discharge plasma excited by bipolar nanosecond pulse in quartz container with different bottom structures at atmospheric pressure. Optical diagnostic measurements show that bountiful chemically and biologically active species, which are beneficial for effective sterilization in some areas, are produced. Such diffuse plasmas are then used to treat drinking water containing the common microorganisms (Candida albicans and Escherichia coli). It is found that these plasmas can sterilize the microorganisms efficiently.

  2. Low-threshold and high efficiency lasing upon band-edge excitation in a cholesteric liquid crystal

    NASA Astrophysics Data System (ADS)

    Matsuhisa, Yuko; Huang, Yuhua; Zhou, Ying; Wu, Shin-Tson; Ozaki, Ryotaro; Takao, Yuuki; Fujii, Akihiko; Ozaki, Masanori

    2007-02-01

    A low threshold and high efficiency laser based on dye-doped cholesteric liquid crystals (CLCs) is demonstrated using an input excitation with the same handedness of circular polarization as the helical structure of the sample at the shorter wavelength band edge of the reflection band. The responsible mechanism originates from the dramatic increase of the optical density of state (DOS) at the band edges. The calculated DOS of the CLC system confirms the authors' experimental results.

  3. Cryogenic exciter

    SciTech Connect

    Bray, James William; Garces, Luis Jose

    2012-03-13

    The disclosed technology is a cryogenic static exciter. The cryogenic static exciter is connected to a synchronous electric machine that has a field winding. The synchronous electric machine is cooled via a refrigerator or cryogen like liquid nitrogen. The static exciter is in communication with the field winding and is operating at ambient temperature. The static exciter receives cooling from a refrigerator or cryogen source, which may also service the synchronous machine, to selected areas of the static exciter and the cooling selectively reduces the operating temperature of the selected areas of the static exciter.

  4. Evolution of the excited electron bubble in liquid H4e and the appearance of fission-like processes

    NASA Astrophysics Data System (ADS)

    Mateo, David; Pi, Martí; Barranco, Manuel

    2010-05-01

    We have studied the evolution of an excited electron bubble in superfluid H4e for several tens of picosecond combining the dynamics of the liquid with an adiabatic evolution for the electron. The path followed by the excited bubble in its decay to the ground state is shown to strongly depend on pressure. While for pressures below 1 bar the 1P excited electron bubble has allowance for radiatively decay to the deformed ground state, evolving then nonradiatively toward the ground state of the spherical electron bubble, we have found that above 1 bar two distinct baby bubbles appear in the course of the dynamical evolution, pointing to a different relaxation path in which the electron may be localized in one of the baby bubbles while the other collapses, allowing for a pure radiationless de-excitation. Our calculations are in agreement with experiments indicating that relaxed 1P bubbles are only observed for pressures smaller than a critical one, on the order of 1 bar, and that above this value the decay of the excited bubble has to proceed differently. A similar analysis carried out for the 2P bubble shows that the adiabatic approximation fails at an early stage of its dynamical evolution due to the crossing of the 2P and 1F states.

  5. Pressure-induced emergence of unusually high-frequency transverse excitations in a liquid alkali metal: Evidence of two types of collective excitations contributing to the transverse dynamics at high pressures

    SciTech Connect

    Bryk, Taras; Ruocco, G.; Scopigno, T.

    2015-09-14

    Unlike phonons in crystals, the collective excitations in liquids cannot be treated as propagation of harmonic displacements of atoms around stable local energy minima. The viscoelasticity of liquids, reflected in transition from the adiabatic to elastic high-frequency speed of sound and in absence of the long-wavelength transverse excitations, results in dispersions of longitudinal (L) and transverse (T) collective excitations essentially different from the typical phonon ones. Practically, nothing is known about the effect of high pressure on the dispersion of collective excitations in liquids, which causes strong changes in liquid structure. Here dispersions of L and T collective excitations in liquid Li in the range of pressures up to 186 GPa were studied by ab initio simulations. Two methodologies for dispersion calculations were used: direct estimation from the peak positions of the L/T current spectral functions and simulation-based calculations of wavenumber-dependent collective eigenmodes. It is found that at ambient pressure, the longitudinal and transverse dynamics are well separated, while at high pressures, the transverse current spectral functions, density of vibrational states, and dispersions of collective excitations yield evidence of two types of propagating modes that contribute strongly to transverse dynamics. Emergence of the unusually high-frequency transverse modes gives evidence of the breakdown of a regular viscoelastic theory of transverse dynamics, which is based on coupling of a single transverse propagating mode with shear relaxation. The explanation of the observed high-frequency shift above the viscoelastic value is given by the presence of another branch of collective excitations. With the pressure increasing, coupling between the two types of collective excitations is rationalized within a proposed extended viscoelastic model of transverse dynamics.

  6. Minimal-excitation states for electron quantum optics using levitons.

    PubMed

    Dubois, J; Jullien, T; Portier, F; Roche, P; Cavanna, A; Jin, Y; Wegscheider, W; Roulleau, P; Glattli, D C

    2013-10-31

    The on-demand generation of pure quantum excitations is important for the operation of quantum systems, but it is particularly difficult for a system of fermions. This is because any perturbation affects all states below the Fermi energy, resulting in a complex superposition of particle and hole excitations. However, it was predicted nearly 20 years ago that a Lorentzian time-dependent potential with quantized flux generates a minimal excitation with only one particle and no hole. Here we report that such quasiparticles (hereafter termed levitons) can be generated on demand in a conductor by applying voltage pulses to a contact. Partitioning the excitations with an electronic beam splitter generates a current noise that we use to measure their number. Minimal-excitation states are observed for Lorentzian pulses, whereas for other pulse shapes there are significant contributions from holes. Further identification of levitons is provided in the energy domain with shot-noise spectroscopy, and in the time domain with electronic Hong-Ou-Mandel noise correlations. The latter, obtained by colliding synchronized levitons on a beam splitter, exemplifies the potential use of levitons for quantum information: using linear electron quantum optics in ballistic conductors, it is possible to imagine flying-qubit operation in which the Fermi statistics are exploited to entangle synchronized electrons emitted by distinct sources. Compared with electron sources based on quantum dots, the generation of levitons does not require delicate nanolithography, considerably simplifying the circuitry for scalability. Levitons are not limited to carrying a single charge, and so in a broader context n-particle levitons could find application in the study of full electron counting statistics. But they can also carry a fraction of charge if they are implemented in Luttinger liquids or in fractional quantum Hall edge channels; this allows the study of Abelian and non-Abelian quasiparticles in the

  7. Minimal-excitation states for electron quantum optics using levitons

    NASA Astrophysics Data System (ADS)

    Dubois, J.; Jullien, T.; Portier, F.; Roche, P.; Cavanna, A.; Jin, Y.; Wegscheider, W.; Roulleau, P.; Glattli, D. C.

    2013-10-01

    The on-demand generation of pure quantum excitations is important for the operation of quantum systems, but it is particularly difficult for a system of fermions. This is because any perturbation affects all states below the Fermi energy, resulting in a complex superposition of particle and hole excitations. However, it was predicted nearly 20 years ago that a Lorentzian time-dependent potential with quantized flux generates a minimal excitation with only one particle and no hole. Here we report that such quasiparticles (hereafter termed levitons) can be generated on demand in a conductor by applying voltage pulses to a contact. Partitioning the excitations with an electronic beam splitter generates a current noise that we use to measure their number. Minimal-excitation states are observed for Lorentzian pulses, whereas for other pulse shapes there are significant contributions from holes. Further identification of levitons is provided in the energy domain with shot-noise spectroscopy, and in the time domain with electronic Hong-Ou-Mandel noise correlations. The latter, obtained by colliding synchronized levitons on a beam splitter, exemplifies the potential use of levitons for quantum information: using linear electron quantum optics in ballistic conductors, it is possible to imagine flying-qubit operation in which the Fermi statistics are exploited to entangle synchronized electrons emitted by distinct sources. Compared with electron sources based on quantum dots, the generation of levitons does not require delicate nanolithography, considerably simplifying the circuitry for scalability. Levitons are not limited to carrying a single charge, and so in a broader context n-particle levitons could find application in the study of full electron counting statistics. But they can also carry a fraction of charge if they are implemented in Luttinger liquids or in fractional quantum Hall edge channels; this allows the study of Abelian and non-Abelian quasiparticles in the

  8. YIELDS OF IONS AND EXCITED STATES IN NONPOLAR LIQUIDS EXPOSED TO X-RAYS OF 1 TO 30 KEV ENERGY

    SciTech Connect

    HOLROYD,R.A.

    1999-08-18

    When x-rays from a synchrotron source are absorbed in a liquid, the x-ray energy (E{sub x}) is converted by the photoelectric effect into the kinetic energy of the electrons released. For hydrocarbons, absorption by the K-electrons of carbon dominates. Thus the energy of the photoelectron (E{sub pe}) is E{sub x}-E{sub b}, where E{sub b} is the K-shell binding energy of carbon. Additional electrons with energy equal to E{sub b} is released in the Auger process that fills the hole in the K-shell. These energetic electrons will produce many ionizations, excitations and products. The consequences of the high density of ionizations and excitations along the track of the photoelectron and special effects near the K-edge are examined here.

  9. Focus: Phase-resolved nonlinear terahertz spectroscopy—From charge dynamics in solids to molecular excitations in liquids

    SciTech Connect

    Elsaesser, Thomas Reimann, Klaus; Woerner, Michael

    2015-06-07

    Intense terahertz (THz) electric field transients with amplitudes up to several megavolts/centimeter and novel multidimensional techniques are the key ingredients of nonlinear THz spectroscopy, a new area of basic research. Both nonlinear light-matter interactions including the non-perturbative regime and THz driven charge transport give new insight into the character and dynamics of low-energy excitations of condensed matter and into quantum kinetic phenomena. This article provides an overview of recent progress in this field, combining an account of technological developments with selected prototype results for liquids and solids. The potential of nonlinear THz methods for future studies of low-frequency excitations of condensed-phase molecular systems is discussed as well.

  10. The fluorescence action spectra of some saturated hydrocarbon liquids for excitation energies above and below their ionization thresholds

    SciTech Connect

    Ostafin, A.E.; Lipsky, S. )

    1993-04-01

    Fluorescence action spectra have been obtained for the neat liquids, [ital cis]-decalin, [ital trans]-decalin, bicyclohexyl, cyclohexane, methylcyclohexane, isobutylcyclohexane, 2,3,4-trimethylpentane, 2,3-dimethylbutane, 3-methylhexane, 3-methylpentane, [ital n]-decane, [ital n]-dodecane, and [ital n]-pentadecane at excitation energies, [epsilon], ranging from their absorption onsets (at ca. 7 eV) to 10.3 eV. For all compounds, with the exception of [ital cis]-decalin, the fluorescence quantum yield is observed to monotonically decline with increasing [epsilon], reaching a minimum value at an energy, [epsilon][sub [ital m

  11. Multifrequency force microscopy using flexural and torsional modes by photothermal excitation in liquid: atomic resolution imaging of calcite (1014).

    PubMed

    Meier, Tobias; Eslami, Babak; Solares, Santiago D

    2016-02-26

    We introduce a new multifrequency atomic force microscopy (AFM) method which involves the excitation of flexural and torsional eigenmodes of the microcantilever probe in liquid environments. The flexural and torsional deflection signals are mostly decoupled in the majority of commercial AFM setups, so they can be relatively easily recorded and processed. The use of torsional modes provides additional surface information at the atomic scale, with respect to flexural mode imaging alone, although the flexural modes are the only ones capable of 'true' atomic resolution imaging. In our experiments, the torsional modes are shown to be particularly sensitive to protruding oxygen surface atoms on the calcite (1014) plane. The high lateral resolution capability of the flexural modes, combined with the high sensitivity of the torsional modes to specific surface features in liquid environments, can thus offer the means of observing chemical contrast at the atomic level using purely mechanical measurement AFM techniques, even in the absence of tip functionalization. PMID:26807504

  12. Excitation-energy dependence of solvation dynamics in room-temperature ionic liquids

    NASA Astrophysics Data System (ADS)

    Kim, Daekeon; Park, Sang-Won; Shim, Youngseon; Kim, Hyung J.; Jung, YounJoon

    2016-07-01

    Influence of the excitation energy of a probe solute molecule on its solvation dynamics and emission spectrum in 1-ethyl-3-methylimidazolium hexafluorophosphate (EMI+PF6-) is studied via molecular dynamics simulations using a coarse-grained model description. By exciting the probe at different energies, each with an extremely narrow distribution, ensuing solvent relaxation and its dynamic variance are monitored using the isoconfigurational ensemble method. Resulting Stokes shift function, S(t), indicates that long-time solvent relaxation becomes slower with the decreasing excitation energy and approaches the equilibrium correlation function, C(t), of solvent fluctuations. This suggests that the system excited at the red-edge of the spectrum observes linear response better than that at the blue-edge. A detailed analysis of nonequilibrium trajectories shows that the effect of initial configurations on variance of relaxation dynamics is mainly confined to short times; it reaches a maximum around 0.1 ≲ t ≲ 1 ps and diminishes as time further increases. The influence of the initial velocity distribution, on the other hand, tends to grow with time and dominates the long-time variations of dynamics. The emission spectrum shows the red-edge effect in accord with previous studies.

  13. Excitation-energy dependence of solvation dynamics in room-temperature ionic liquids.

    PubMed

    Kim, Daekeon; Park, Sang-Won; Shim, Youngseon; Kim, Hyung J; Jung, YounJoon

    2016-07-28

    Influence of the excitation energy of a probe solute molecule on its solvation dynamics and emission spectrum in 1-ethyl-3-methylimidazolium hexafluorophosphate (EMI(+)PF6 (-)) is studied via molecular dynamics simulations using a coarse-grained model description. By exciting the probe at different energies, each with an extremely narrow distribution, ensuing solvent relaxation and its dynamic variance are monitored using the isoconfigurational ensemble method. Resulting Stokes shift function, S(t), indicates that long-time solvent relaxation becomes slower with the decreasing excitation energy and approaches the equilibrium correlation function, C(t), of solvent fluctuations. This suggests that the system excited at the red-edge of the spectrum observes linear response better than that at the blue-edge. A detailed analysis of nonequilibrium trajectories shows that the effect of initial configurations on variance of relaxation dynamics is mainly confined to short times; it reaches a maximum around 0.1 ≲ t ≲ 1 ps and diminishes as time further increases. The influence of the initial velocity distribution, on the other hand, tends to grow with time and dominates the long-time variations of dynamics. The emission spectrum shows the red-edge effect in accord with previous studies.

  14. Influence of an amorphous wall on the distribution of localized excitations in a colloidal glass-forming liquid

    NASA Astrophysics Data System (ADS)

    Gokhale, Shreyas; Hima Nagamanasa, K.; Sood, A. K.; Ganapathy, Rajesh

    2016-07-01

    Elucidating the nature of the glass transition has been the holy grail of condensed matter physics and statistical mechanics for several decades. A phenomenological aspect that makes glass formation a conceptually formidable problem is that structural and dynamic correlations in glass-forming liquids are too subtle to be captured at the level of conventional two-point functions. As a consequence, a host of theoretical techniques, such as quenched amorphous configurations of particles, have been devised and employed in simulations and colloid experiments to gain insights into the mechanisms responsible for these elusive correlations. Very often, though, the analysis of spatio-temporal correlations is performed in the context of a single theoretical framework, and critical comparisons of microscopic predictions of competing theories are thereby lacking. Here, we address this issue by analysing the distribution of localized excitations, which are building blocks of relaxation as per the dynamical facilitation (DF) theory, in the presence of an amorphous wall, a construct motivated by the random first-order transition theory (RFOT). We observe that spatial profiles of the concentration of excitations exhibit complex features such as non-monotonicity and oscillations. Moreover, the smoothly varying part of the concentration profile yields a length scale {ξc} , which we compare with a previously computed length scale {ξ\\text{dyn}} . Our results suggest a method to assess the role of dynamical facilitation in governing structural relaxation in glass-forming liquids.

  15. Correcting spherical aberrations in a biospecimen using a transmissive liquid crystal device in two-photon excitation laser scanning microscopy

    NASA Astrophysics Data System (ADS)

    Tanabe, Ayano; Hibi, Terumasa; Ipponjima, Sari; Matsumoto, Kenji; Yokoyama, Masafumi; Kurihara, Makoto; Hashimoto, Nobuyuki; Nemoto, Tomomi

    2015-10-01

    Two-photon excitation laser scanning microscopy has enabled the visualization of deep regions in a biospecimen. However, refractive-index mismatches in the optical path cause spherical aberrations that degrade spatial resolution and the fluorescence signal, especially during observation at deeper regions. Recently, we developed transmissive liquid-crystal devices for correcting spherical aberration without changing the basic design of the optical path in a conventional laser scanning microscope. In this study, the device was inserted in front of the objective lens and supplied with the appropriate voltage according to the observation depth. First, we evaluated the device by observing fluorescent beads in single- and two-photon excitation laser scanning microscopes. Using a 25× water-immersion objective lens with a numerical aperture of 1.1 and a sample with a refractive index of 1.38, the device recovered the spatial resolution and the fluorescence signal degraded within a depth of ±0.6 mm. Finally, we implemented the device for observation of a mouse brain slice in a two-photon excitation laser scanning microscope. An optical clearing reagent with a refractive index of 1.42 rendered the fixed mouse brain transparent. The device improved the spatial resolution and the yellow fluorescent protein signal within a depth of 0-0.54 mm.

  16. Correcting spherical aberrations in a biospecimen using a transmissive liquid crystal device in two-photon excitation laser scanning microscopy.

    PubMed

    Tanabe, Ayano; Hibi, Terumasa; Ipponjima, Sari; Matsumoto, Kenji; Yokoyama, Masafumi; Kurihara, Makoto; Hashimoto, Nobuyuki; Nemoto, Tomomi

    2015-10-01

    Two-photon excitation laser scanning microscopy has enabled the visualization of deep regions in a biospecimen. However, refractive-index mismatches in the optical path cause spherical aberrations that degrade spatial resolution and the fluorescence signal, especially during observation at deeper regions. Recently, we developed transmissive liquid-crystal devices for correcting spherical aberration without changing the basic design of the optical path in a conventional laser scanning microscope. In this study, the device was inserted in front of the objective lens and supplied with the appropriate voltage according to the observation depth. First, we evaluated the device by observing fluorescent beads in single- and two-photon excitation laser scanning microscopes. Using a 25× water-immersion objective lens with a numerical aperture of 1.1 and a sample with a refractive index of 1.38, the device recovered the spatial resolution and the fluorescence signal degraded within a depth of 0.6 mm. Finally, we implemented the device for observation of a mouse brain slice in a two-photon excitation laser scanning microscope. An optical clearing reagent with a refractive index of 1.42 rendered the fixed mouse brain transparent. The device improved the spatial resolution and the yellow fluorescent protein signal within a depth of 0-0.54 mm. PMID:26244766

  17. Correcting spherical aberrations in a biospecimen using a transmissive liquid crystal device in two-photon excitation laser scanning microscopy.

    PubMed

    Tanabe, Ayano; Hibi, Terumasa; Ipponjima, Sari; Matsumoto, Kenji; Yokoyama, Masafumi; Kurihara, Makoto; Hashimoto, Nobuyuki; Nemoto, Tomomi

    2015-10-01

    Two-photon excitation laser scanning microscopy has enabled the visualization of deep regions in a biospecimen. However, refractive-index mismatches in the optical path cause spherical aberrations that degrade spatial resolution and the fluorescence signal, especially during observation at deeper regions. Recently, we developed transmissive liquid-crystal devices for correcting spherical aberration without changing the basic design of the optical path in a conventional laser scanning microscope. In this study, the device was inserted in front of the objective lens and supplied with the appropriate voltage according to the observation depth. First, we evaluated the device by observing fluorescent beads in single- and two-photon excitation laser scanning microscopes. Using a 25× water-immersion objective lens with a numerical aperture of 1.1 and a sample with a refractive index of 1.38, the device recovered the spatial resolution and the fluorescence signal degraded within a depth of 0.6 mm. Finally, we implemented the device for observation of a mouse brain slice in a two-photon excitation laser scanning microscope. An optical clearing reagent with a refractive index of 1.42 rendered the fixed mouse brain transparent. The device improved the spatial resolution and the yellow fluorescent protein signal within a depth of 0-0.54 mm.

  18. Determination of leucomalachite green, leucocrystal violet and their chromic forms using excitation-emission matrix fluorescence coupled with second-order calibration after dispersive liquid-liquid microextraction.

    PubMed

    Ju, Saiqin; Deng, Jian; Cheng, Jianlin; Xiao, Ni; Huang, Kaihui; Hu, Canhui; Zhao, Haiqing; Xie, Jin; Zhan, Xiaozhu

    2015-10-15

    A novel spectrofluorimetric method has been developed for the simultaneous determination of leucomalachite green (LMG), leucocrystal violet (LCV), malachite green (MG) and crystal violet (CV) by combining the sensitivity of molecular fluorescence and the selectivity of the second-order calibration. Residues of LMG, LCV, MG and CV were simultaneously extracted from fish and shrimp muscle with acetonitrile. The non-fluorescent CV and MG were then reduced to the corresponding fluorescent LMG and LCV by reacting with sodium borohydride. After preconcentration with dispersive liquid-liquid microextraction technique, the extracts were analyzed by using excitation-emission matrix fluorescence coupled with second-order calibration methods based on parallel factor analysis (PARAFAC) and alternating trilinear decomposition (ATLD) algorithms. The limits of detection obtained were 2.21-2.65 ng g(-1) by PARAFAC and 2.30-2.86 ng g(-1) by ATLD, respectively. The developed method was successfully applied to simultaneous determination of the four analytes in grass carp and shrimp samples with recoveries of 90.53-103.03% for PARAFAC and 90.40-102.75% for ATLD. The accuracy of this novel method was also verified by high performance liquid chromatography. PMID:25952896

  19. Kohn-Luttinger superconductivity in monolayer and bilayer semimetals with the Dirac spectrum

    NASA Astrophysics Data System (ADS)

    Kagan, M. Yu.; Mitskan, V. A.; Korovushkin, M. M.

    2014-12-01

    The effect of Coulomb interaction in an ensemble of Dirac fermions on the formation of superconducting pairing in monolayer and bilayer doped graphene is studied using the Kohn-Luttinger mechanism disregarding the Van der Waals potential of the substrate and impurities. The electronic structure of graphene is described using the Shubin-Vonsovsky model taking into account the intratomic, interatomic, and interlayer (in the case of bilayer graphene) Coulomb interactions between electrons. The Cooper instability is determined by solving the Bethe-Saltpeter integral equation. The renormalized scattering amplitude is obtained with allowance for the Kohn-Luttinger polarization contributions up to the second order of perturbation theory in the Coulomb interaction. It plays the role of effective interaction in the Bethe-Salpeter integral equation. It is shown that the allowance for the Kohn-Luttinger renormalizations as well as intersite Coulomb interaction noticeably affects the competition between the superconducting phases with the f-wave and d + id-wave symmetries of the order parameter. It is demonstrated that the superconducting transition temperature for an idealized graphene bilayer with significant interlayer Coulomb interaction between electrons is noticeably higher than in the monolayer case.

  20. Kohn-Luttinger superconductivity in monolayer and bilayer semimetals with the Dirac spectrum

    SciTech Connect

    Kagan, M. Yu.; Mitskan, V. A.; Korovushkin, M. M.

    2014-12-15

    The effect of Coulomb interaction in an ensemble of Dirac fermions on the formation of superconducting pairing in monolayer and bilayer doped graphene is studied using the Kohn-Luttinger mechanism disregarding the Van der Waals potential of the substrate and impurities. The electronic structure of graphene is described using the Shubin-Vonsovsky model taking into account the intratomic, interatomic, and interlayer (in the case of bilayer graphene) Coulomb interactions between electrons. The Cooper instability is determined by solving the Bethe-Saltpeter integral equation. The renormalized scattering amplitude is obtained with allowance for the Kohn-Luttinger polarization contributions up to the second order of perturbation theory in the Coulomb interaction. It plays the role of effective interaction in the Bethe-Salpeter integral equation. It is shown that the allowance for the Kohn-Luttinger renormalizations as well as intersite Coulomb interaction noticeably affects the competition between the superconducting phases with the f-wave and d + id-wave symmetries of the order parameter. It is demonstrated that the superconducting transition temperature for an idealized graphene bilayer with significant interlayer Coulomb interaction between electrons is noticeably higher than in the monolayer case.

  1. Photo-excited states in germanium at liquid-helium temperatures

    SciTech Connect

    Culbertson, J.C.

    1982-12-01

    A wide variety of experimental work dealing with the basic properties of photoexcited states in Ge at liquid helium temperatures is presented. The primary emphasis is on the electron-hole liquid (EHL) and the free exciton (FE). The EHL is composed of two interpenetrating Fermi liquids, one of electrons and one of holes, each with its own Fermi level. The FE dealt with here is a mobile, loosely bound state of an electron and a hole. We report the first absolute measurement of the density dependence of the enhancement factor g/sub eh/(0) for the EHL in Ge. This factor g/sub eh/(0) is a measure of the electron-hole spatial correlation function, and provides a valuable and sensitive test for the predictions of various many-body-theory approximations. An EHL droplet - FE gas system confined to a strain induced potential well was used. The measurement approach relied on only a few simple and verifiable assumptions. A byproduct of this work was the measurement as a function of stress of: the electron and hole Fermi levels E/sub F//sup e/ and E/sub F//sup h/, the EHL density n/sub l/, the condensation energy phi of a FE relative to the EHL, and the binding energy of a FE (E/sub x/) relative to free carriers (FC). The decay of a FE-FC system confined to a strain induced potential well is studied. The first direct measurement of the FE diffusivity D/sub x/ is reported. The evolution in time of spatial profiles of FE luminescence were measured. From these FE density profiles, D/sub x/(4.2K) approx. = to 300 cm/sup 2/ s/sup -1/, the surface recombination velocity S approx. = 3000 cm s/sup -1/, and the FE lifetime tau/sub x/ = 27 ..mu..s with surface effects excluded were determined. (WHK)

  2. Transient, polarity-dependent dielectric response in a twisted nematic liquid crystal under very low frequency excitation.

    PubMed

    Krishnamurthy, K S

    2015-09-01

    The electric Freedericksz transition is a second-order quadratic effect, which, in a planarly aligned nematic liquid crystal layer, manifests above a threshold field as a homogeneous symmetric distortion with maximum director-tilt in the midplane. We find that, upon excitation by a low frequency (<0.2Hz) square-wave field, the instability becomes spatially and temporally varying. This is demonstrated using calamitic liquid crystals, initially in the 90°-twisted planar configuration. The distortion occurs close to the negative electrode following each polarity switch and, for low-voltage amplitudes, decays completely in time. We use the elastically favorable geometry of Brochard-Leger walls to establish the location of maximum distortion. Thus, at successive polarity changes, the direction of extension of both annular and open walls switches between the alignment directions at the two substrates. For high voltages, this direction is largely along the midplane director, while remaining marginally oscillatory. These results are broadly understood by taking into account the time-varying and inhomogeneous field conditions that prevail soon after the polarity reverses. Polarity dependence of the instability is traced to the formation of intrinsic double layers that lead to an asymmetry in field distribution in the presence of an external bias. Momentary field elevation near the negative electrode following a voltage sign reversal leads to locally enhanced dielectric and gradient flexoelectric torques, which accounts for the surface-like phenomenon observed at low voltages. These spatiotemporal effects, also found earlier for other instabilities, are generic in nature.

  3. Spiral and target patterns in bivalve nacre manifest a natural excitable medium from layer growth of a biological liquid crystal

    PubMed Central

    Cartwright, Julyan H. E.; Checa, Antonio G.; Escribano, Bruno; Sainz-Díaz, C. Ignacio

    2009-01-01

    Nacre is an exquisitely structured biocomposite of the calcium carbonate mineral aragonite with small amounts of proteins and the polysaccharide chitin. For many years, it has been the subject of research, not just because of its beauty, but also to discover how nature can produce such a superior product with excellent mechanical properties from such relatively weak raw materials. Four decades ago, Wada [Wada K (1966) Spiral growth of nacre. Nature 211:1427] proposed that the spiral patterns in nacre could be explained by using the theory Frank [Frank F (1949) The influence of dislocations on crystal growth. Discuss Faraday Soc 5:48–54] had put forward of the growth of crystals by means of screw dislocations. Frank's mechanism of crystal growth has been amply confirmed by experimental observations of screw dislocations in crystals, but it is a growth mechanism for a single crystal, with growth fronts of molecules. However, the growth fronts composed of many tablets of crystalline aragonite visible in micrographs of nacre are not a molecular-scale but a mesoscale phenomenon, so it has not been evident how the Frank mechanism might be of relevance. Here, we demonstrate that nacre growth is organized around a liquid-crystal core of chitin crystallites, a skeleton that the other components of nacre subsequently flesh out in a process of hierarchical self-assembly. We establish that spiral and target patterns can arise in a liquid crystal formed layer by layer through the Burton–Cabrera–Frank [Burton W, Cabrera N, Frank F (1951) The growth of crystals and the equilibrium structure of their surfaces. Philos Trans R Soc London Ser A 243:299–358] dynamics, and furthermore that this layer growth mechanism is an instance of an important class of physical systems termed excitable media. Artificial liquid crystals grown in this way may have many technological applications. PMID:19528636

  4. Spiral and target patterns in bivalve nacre manifest a natural excitable medium from layer growth of a biological liquid crystal.

    PubMed

    Cartwright, Julyan H E; Checa, Antonio G; Escribano, Bruno; Sainz-Díaz, C Ignacio

    2009-06-30

    Nacre is an exquisitely structured biocomposite of the calcium carbonate mineral aragonite with small amounts of proteins and the polysaccharide chitin. For many years, it has been the subject of research, not just because of its beauty, but also to discover how nature can produce such a superior product with excellent mechanical properties from such relatively weak raw materials. Four decades ago, Wada [Wada K (1966) Spiral growth of nacre. Nature 211:1427] proposed that the spiral patterns in nacre could be explained by using the theory Frank [Frank F (1949) The influence of dislocations on crystal growth. Discuss Faraday Soc 5:48-54] had put forward of the growth of crystals by means of screw dislocations. Frank's mechanism of crystal growth has been amply confirmed by experimental observations of screw dislocations in crystals, but it is a growth mechanism for a single crystal, with growth fronts of molecules. However, the growth fronts composed of many tablets of crystalline aragonite visible in micrographs of nacre are not a molecular-scale but a mesoscale phenomenon, so it has not been evident how the Frank mechanism might be of relevance. Here, we demonstrate that nacre growth is organized around a liquid-crystal core of chitin crystallites, a skeleton that the other components of nacre subsequently flesh out in a process of hierarchical self-assembly. We establish that spiral and target patterns can arise in a liquid crystal formed layer by layer through the Burton-Cabrera-Frank [Burton W, Cabrera N, Frank F (1951) The growth of crystals and the equilibrium structure of their surfaces. Philos Trans R Soc London Ser A 243:299-358] dynamics, and furthermore that this layer growth mechanism is an instance of an important class of physical systems termed excitable media. Artificial liquid crystals grown in this way may have many technological applications.

  5. Electronic excited states as a probe of surface adsorbate structure and dynamics in liquid xenon

    SciTech Connect

    Peterson, E.S.

    1992-08-01

    A combination of second harmonic generation (SHG) and a simple dipole-dipole interaction model is presented as a new technique for determining adsorbate geometries on surfaces. The polarization dependence of SHG is used to define possible geometries of the adsorbate about the surface normal. Absorption band shifts using geometry constraints imposed by SHG data are derived for a dimer constructed from two arbitrarily placed monomers on the surface using the dipole-dipole interaction potential. These formulae can be used to determine the orientation of the two monomers relative to each other. A simplified version of this formalism is used to interpret absorption band shifts for rhodamine B adsorbed on fused silica. A brief history of the exciton is given with particular detail to Xe. Data are presented for transient absorption at RT in liquid xenon on the picosecond time scale. These are observations of both tunneling through the barrier that separates the free and trapped exciton states and the subsequent trapping of the exciton. In high densities both of these processes are found to occur within 2 to 6 picoseconds in agreement with theories of Kmiecik and Schreiber and of Martin. A threshold density is observed that separates relaxation via single binary collisions and relaxation that proceeds via Martin`s resonant energy transfer hopping mechanism.

  6. Electronic excited states as a probe of surface adsorbate structure and dynamics in liquid xenon

    SciTech Connect

    Peterson, E.S.

    1992-08-01

    A combination of second harmonic generation (SHG) and a simple dipole-dipole interaction model is presented as a new technique for determining adsorbate geometries on surfaces. The polarization dependence of SHG is used to define possible geometries of the adsorbate about the surface normal. Absorption band shifts using geometry constraints imposed by SHG data are derived for a dimer constructed from two arbitrarily placed monomers on the surface using the dipole-dipole interaction potential. These formulae can be used to determine the orientation of the two monomers relative to each other. A simplified version of this formalism is used to interpret absorption band shifts for rhodamine B adsorbed on fused silica. A brief history of the exciton is given with particular detail to Xe. Data are presented for transient absorption at RT in liquid xenon on the picosecond time scale. These are observations of both tunneling through the barrier that separates the free and trapped exciton states and the subsequent trapping of the exciton. In high densities both of these processes are found to occur within 2 to 6 picoseconds in agreement with theories of Kmiecik and Schreiber and of Martin. A threshold density is observed that separates relaxation via single binary collisions and relaxation that proceeds via Martin's resonant energy transfer hopping mechanism.

  7. Superdeformed nuclei: Shells-vs-liquid drop, pairing-vs-thermal excitations, triaxial-vs-octupole shapes, super-superdeformation

    SciTech Connect

    Dudek, J.

    1987-01-01

    Mechanisms influencing the behavior of superdeformed nuclei are studied using several well established nuclear structure techniques. In particular: pairing, thermal excitation, shell and liquid-drop mechanisms are considered. The effects of quadrupole and hexadecapole (both axial and non-axial), and octupole deformation degrees of freedom are studied. Most of the results are illustrated using the case of /sup 152/Dy nucleus in which a superdeformed band extending up to I approx. 60 h-bar has been found in experiment. Some comparisons between /sup 152/Dy and the nuclei in the neighborhood are given. Calculations show that pairing ''de-aligns'' typically 6 to 8 units of angular momentum, as compared to the corresponding rigid rotation. This takes place for spins extending up to the highest limit, and thus diminishes the effective moments of inertia. Predicted octupole shape susceptibility is extremely large, significantly stronger than the susceptibilities known in the ground-states of many Actinide nuclei. Consequences of this result for the near-constancy of the dynamical moments of inertia are pointed out. Nuclear level densities calculated in function of spin, excitation energy and deformation explain the ''unusual'' side feeding pattern of the /sup 152/Dy superdeformed states. Predictions of super-superdeformed nuclear states (axis ratio varying between 2:1 and 3:1 or more) are given and exemplified for Erbium nuclei. Finally, the problem of superdeformation stability and the influence of increased collective inertia on a barrier penetration are examined. An analytical expression for the effective inertia parameter is obtained and its derivation outlined. 35 refs., 9 figs.

  8. Excitation spectra and correlation functions of quantum Su-Schrieffer-Heeger models

    NASA Astrophysics Data System (ADS)

    Weber, Manuel; Assaad, Fakher F.; Hohenadler, Martin

    2015-06-01

    We study one-dimensional Su-Schrieffer-Heeger (SSH) models with quantum phonons using a continuous-time quantum Monte Carlo method. Within statistical errors, we obtain identical results for the SSH model with acoustic phonons, and a related model with a coupling to an optical bond phonon mode. Based on this agreement, we first study the Peierls metal-insulator transition of the spinless SSH model, and relate it to the Kosterlitz-Thouless transition of a spinless Luttinger liquid. In the Peierls phase, the spectral functions reveal the single-particle and charge gap, and a central peak related to long-range order. For the spinful SSH model, which has a dimerized ground state for any nonzero coupling, we reveal a symmetry-related degeneracy of spin and charge excitations, and the expected spin and charge gaps as well as a central peak. Finally, we study the SSH-U V model with electron-phonon and electron-electron interaction. We observe a Mott phase with critical spin and bond correlations at weak electron-phonon coupling, and a Peierls phase with gapped spin excitations at strong coupling. We relate our findings to the extended Hubbard model, and discuss the physical origin of the agreement between optical and acoustic phonons.

  9. Transient, polarity-dependent dielectric response in a twisted nematic liquid crystal under very low frequency excitation.

    PubMed

    Krishnamurthy, K S

    2015-09-01

    The electric Freedericksz transition is a second-order quadratic effect, which, in a planarly aligned nematic liquid crystal layer, manifests above a threshold field as a homogeneous symmetric distortion with maximum director-tilt in the midplane. We find that, upon excitation by a low frequency (<0.2Hz) square-wave field, the instability becomes spatially and temporally varying. This is demonstrated using calamitic liquid crystals, initially in the 90°-twisted planar configuration. The distortion occurs close to the negative electrode following each polarity switch and, for low-voltage amplitudes, decays completely in time. We use the elastically favorable geometry of Brochard-Leger walls to establish the location of maximum distortion. Thus, at successive polarity changes, the direction of extension of both annular and open walls switches between the alignment directions at the two substrates. For high voltages, this direction is largely along the midplane director, while remaining marginally oscillatory. These results are broadly understood by taking into account the time-varying and inhomogeneous field conditions that prevail soon after the polarity reverses. Polarity dependence of the instability is traced to the formation of intrinsic double layers that lead to an asymmetry in field distribution in the presence of an external bias. Momentary field elevation near the negative electrode following a voltage sign reversal leads to locally enhanced dielectric and gradient flexoelectric torques, which accounts for the surface-like phenomenon observed at low voltages. These spatiotemporal effects, also found earlier for other instabilities, are generic in nature. PMID:26465487

  10. Nucleon effective E-mass in neutron-rich matter from the Migdal-Luttinger jump

    NASA Astrophysics Data System (ADS)

    Cai, Bao-Jun; Li, Bao-An

    2016-06-01

    The well-known Migdal-Luttinger theorem states that the jump of the single-nucleon momentum distribution at the Fermi surface is equal to the inverse of the nucleon effective E-mass. Recent experiments studying short-range correlations (SRC) in nuclei using electron-nucleus scatterings at the Jefferson National Laboratory (JLAB) together with model calculations constrained significantly the Migdal-Luttinger jump at saturation density of nuclear matter. We show that the corresponding nucleon effective E-mass is consequently constrained to M0*,E / M ≈ 2.22 ± 0.35 in symmetric nuclear matter (SNM) and the E-mass of neutrons is smaller than that of protons in neutron-rich matter. Moreover, the average depletion of the nucleon Fermi sea increases (decreases) approximately linearly with the isospin asymmetry δ according to κp/n ≈ 0.21 ± 0.06 ± (0.19 ± 0.08) δ for protons (neutrons). These results will help improve our knowledge about the space-time non-locality of the single-nucleon potential in neutron-rich nucleonic matter useful in both nuclear physics and astrophysics.

  11. Pulsed photoconductivity in diamond upon quasi-continuous laser excitation at 222 nm at the formation of an electron-hole liquid

    NASA Astrophysics Data System (ADS)

    Lipatov, E. I.; Genin, D. E.; Tarasenko, V. F.

    2016-06-01

    An order-of-magnitude enhancement of the pulsed photocurrent in a polycrystalline diamond sample synthesized by chemical vapor deposition is observed under the conditions of formation of an electron-hole liquid. Nonequilibrium charge carriers are excited by laser pulses at a wavelength of 222 nm with FWHM pulse duration of 18 ns and peak intensity above 2.5 MW/cm2 upon cooling the sample to 90 K. For peak intensities of laser excitation lower than 1 MW/cm2, sample cooling from 300 to 90 K leads to a decrease in pulsed photocurrent by about a factor of 5. The observed increase in pulsed photocurrent is attributed to the formation of the electron-hole liquid.

  12. Deuterium isotope effect on femtosecond solvation dynamics in an ionic liquid microemulsion: an excitation wavelength dependence study.

    PubMed

    Sasmal, Dibyendu Kumar; Mojumdar, Supratik Sen; Adhikari, Aniruddha; Bhattacharyya, Kankan

    2010-04-01

    The deuterium isotope effect on the solvation dynamics and the anisotropy decay of coumarin 480 (C480) in a room temperature ionic liquid (RTIL) microemulsion is studied by femtosecond up-conversion. The microemulsion consists of the RTIL 1-pentyl-3-methyl-imidazolium tetra-fluoroborate ([pmim][BF(4)]) in triton X-100 (TX-100)/benzene. Replacement of H(2)O by D(2)O in the microemulsion causes retardation of solvation dynamics. The average solvation time of C480 (tau(s)) in RTIL microemulsion with 5 wt % D(2)O is approximately 1.5-1.7 times slower compared to that in the H(2)O containing RTIL microemulsion. This suggests that the main species in the microemulsion responsible for solvation is the water molecules. In both D(2)O and H(2)O containing RTIL microemulsion, the solvation dynamics exhibits marked dependence on the excitation wavelength (lambda(ex)) and becomes about 15 times faster as lambda(ex) increases from 375 to 435 nm. This is ascribed to the structural heterogeneity in the RTIL microemulsion. For lambda(ex) = 375 nm, the region near the TX-100 surfactant is probed where bound water molecules cause slow solvation dynamics. At 435 nm, the RTIL pool is selected where the water molecules are more mobile and hence gives rise to faster solvation. The average time constant of anisotropy decay shows opposite dependence on lambda(ex) and increases about 2.5-fold from 180 ps at lambda(ex) = 375 nm to 500 ps at lambda(ex) = 435 nm for D(2)O containing RTIL microemulsion. The slower anisotropy decay at lambda(ex) = 435 nm is ascribed to the higher viscosity of RTIL which causes greater friction at the core. PMID:20235504

  13. Time-dependent density functional theory study on the electronic excited-state hydrogen bonding of the chromophore coumarin 153 in a room-temperature ionic liquid.

    PubMed

    Wang, Dandan; Hao, Ce; Wang, Se; Dong, Hong; Qiu, Jieshan

    2012-03-01

    In the present work, in order to investigate the electronic excited-state intermolecular hydrogen bonding between the chromophore coumarin 153 (C153) and the room-temperature ionic liquid N,N-dimethylethanolammonium formate (DAF), both the geometric structures and the infrared spectra of the hydrogen-bonded complex C153-DAF(+) in the excited state were studied by a time-dependent density functional theory (TDDFT) method. We theoretically demonstrated that the intermolecular hydrogen bond C(1) = O(1)···H(1)-O(3) in the hydrogen-bonded C153-DAF(+) complex is significantly strengthened in the S(1) state by monitoring the spectral shifts of the C=O group and O-H group involved in the hydrogen bond C(1) = O(1)···H(1)-O(3). Moreover, the length of the hydrogen bond C(1) = O(1)···H(1)-O(3) between the oxygen atom and hydrogen atom decreased from 1.693 Å to 1.633 Å upon photoexcitation. This was also confirmed by the increase in the hydrogen-bond binding energy from 69.92 kJ mol(-1) in the ground state to 90.17 kJ mol(-1) in the excited state. Thus, the excited-state hydrogen-bond strengthening of the coumarin chromophore in an ionic liquid has been demonstrated theoretically for the first time.

  14. Singlet-triplet excitations and long range entanglement in the spin-orbital liquid candidate FeSc2S4

    NASA Astrophysics Data System (ADS)

    Laurita, N. J.; Deisenhofer, J.; Pan, Lidong; Morris, C. M.; Schmidt, M.; Johnsson, M.; Tsurkan, V.,; Loidl, A.; Armitage, N. P.

    2015-03-01

    Theoretical models of the spin-orbital liquid (SOL) FeSc2S4 have predicted it to be in close proximity to a quantum critical point separating a spin-orbital liquid phase from a long-range ordered magnetic phase. Here, we examine the magnetic excitations of FeSc2S4 through time-domain terahertz spectroscopy under an applied magnetic field. At low temperatures an excitation emerges that we attribute to a singlet-triplet excitation from the SOL ground state. A three-fold splitting of this excitation is observed as a function of applied magnetic field. Using experimentally obtained parameters we compare to existing theoretical models to determine FeSc2S4's proximity to the quantum critical point and establish FeSc2S4 as a SOL with long-range entanglement. Work at Johns Hopkins was supported by the Gordon and Betty Moore Foundation through Grant GBMF2628, the DOE-BES through DE-FG02-08ER46544, and the ARCS Foundation.

  15. Luttinger liquid of polarons in one-dimensional boson-fermion mixtures.

    PubMed

    Mathey, L; Wang, D-W; Hofstetter, W; Lukin, M D; Demler, Eugene

    2004-09-17

    We use the bosonization approach to investigate quantum phases of boson-fermion mixtures (BFM) of atoms confined to one dimension by an anisotropic optical lattice. For a BFM with a single species of fermions we find a charge-density wave phase, a fermion pairing phase, and a phase separation regime. We also obtain the rich phase diagram of a BFM with two species of fermions. We demonstrate that these phase diagrams can be understood in terms of polarons, i.e., atoms "dressed" by screening clouds of the other atom species. Techniques to detect the resulting quantum phases are discussed.

  16. Recent research directions in Fribourg: nuclear dynamics in resonances revealed by 2-dimensional EEL spectra, electron collisions with ionic liquids and electronic excitation of pyrimidine

    NASA Astrophysics Data System (ADS)

    Allan, Michael; Regeta, Khrystyna; Gorfinkiel, Jimena D.; Mašín, Zdeněk; Grimme, Stefan; Bannwarth, Christoph

    2016-05-01

    The article briefly reviews three subjects recently investigated in Fribourg: (i) electron collisions with surfaces of ionic liquids, (ii) two-dimensional (2D) electron energy loss spectra and (iii) resonances in absolute cross sections for electronic excitation of unsaturated compounds. Electron energy loss spectra of four ionic liquids revealed a number of excited states, including triplet states. A solution of a dye in an ionic liquid showed an energy-loss band of the solute, but not in all ionic liquids. 2D spectra reveal state-to-state information (given resonance to given final state) and are shown to be an interesting means to gain insight into dynamics of nuclear motion in resonances. Absolute cross sections for pyrimidine are reported as a function of scattering angle and as a function of electron energy. They reveal resonant structure which was reproduced very nicely by R-matrix calculations. The calculation provided an assignment of the resonances which reveals common patterns in compounds containing double bonds.

  17. Free electrons and ionic liquids: study of excited states by means of electron-energy loss spectroscopy and the density functional theory multireference configuration interaction method.

    PubMed

    Regeta, Khrystyna; Bannwarth, Christoph; Grimme, Stefan; Allan, Michael

    2015-06-28

    The technique of low energy (0-30 eV) electron impact spectroscopy, originally developed for gas phase molecules, is applied to room temperature ionic liquids (IL). Electron energy loss (EEL) spectra recorded near threshold, by collecting 0-2 eV electrons, are largely continuous, assigned to excitation of a quasi-continuum of high overtones and combination vibrations of low-frequency modes. EEL spectra recorded by collecting 10 eV electrons show predominantly discrete vibrational and electronic bands. The vibrational energy-loss spectra correspond well to IR spectra except for a broadening (∼0.04 eV) caused by the liquid surroundings, and enhanced overtone activity indicating a contribution from resonant excitation mechanism. The spectra of four representative ILs were recorded in the energy range of electronic excitations and compared to density functional theory multireference configuration interaction (DFT/MRCI) calculations, with good agreement. The spectra up to about 8 eV are dominated by π-π* transitions of the aromatic cations. The lowest bands were identified as triplet states. The spectral region 2-8 eV was empty in the case of a cation without π orbitals. The EEL spectrum of a saturated solution of methylene green in an IL band showed the methylene green EEL band at 2 eV, indicating that ILs may be used as a host to study nonvolatile compounds by this technique in the future.

  18. Non-Fermi Liquid Behavior in Quasi-One-Dimensional Li0.9Mo6O17

    SciTech Connect

    Hager, J.; Matzdorf, R.; He, Jian; Jin, Rongying; Mandrus, David; Cazalilla, M.; Plummer, E Ward

    2005-01-01

    We present temperature dependent scanning tunneling spectroscopy data of the quasi-one-dimensional conductor Li{sub 0.9}Mo{sub 6}O{sub 17}. The differential tunneling current in our low-temperature spectra shows a power-law behavior around the Fermi energy, which is expected for a clean Luttinger liquid. The power-law exponent is found to be 0.6. Spectra for a temperature range of 5 to 55 K can be fitted fairly well with a model for tunneling into a Luttinger liquid at the appropriate temperature. A fit with a model based on a zero bias anomaly is significantly worse compared to the Luttinger liquid model. No signature of a phase transition at T = 24 K is observed in our temperature dependent data.

  19. A novel ionic liquid-in-oil microemulsion composed of biologically acceptable components: an excitation wavelength dependent fluorescence resonance energy transfer study.

    PubMed

    Mandal, Sarthak; Ghosh, Surajit; Banerjee, Chiranjib; Kuchlyan, Jagannath; Banik, Debasis; Sarkar, Nilmoni

    2013-03-21

    In this work we have reported the formulation of a novel ionic liquid-in-oil (IL/O) microemulsion where the polar core of the ionic liquid, 1-ethyl-3-methylimidazolium n-butylsulfate ([C2mim][C4SO4]), is stabilized by a mixture of two nontoxic nonionic surfactants, polyoxyethylene sorbitan monooleate (Tween-80) and sorbitan laurate (Span-20), in a biological oil phase of isopropyl myristate (IPM). The formation of the microemulsion droplets has been confirmed from the dynamic light scattering (DLS) and phase behavior study. To assess the dynamic heterogeneity of this tween-based IL/O microemulsion, we have performed an excitation wavelength dependent fluorescence resonance energy transfer (FRET) from coumarin 480 (C480) to rhodamine 6G (R6G). The multiple donor-acceptor (D-A) distances, ∼15, 30, and 45 Å, obtained from the rise times of the acceptor emission in the presence of a donor can be rationalized from the varying distribution of the donor, C480, in the different regions of the microemulsion system. With increasing the excitation wavelength from 375 to 408 nm, the contribution of the rise component of ∼240 ps which results the D-A distance of ∼30 Å increases significantly due to the enhanced contribution of the C480 probe molecules closer to the acceptor in the ionic liquid pool of the microemulsion. PMID:23445434

  20. B{sub 2u} {yields} A{sub 1g} fluorescence excitation spectrum of liquid benzene from 250 to 150 nm

    SciTech Connect

    Saik, V.O.; Lipsky, S.

    1995-06-29

    The B{sub 2u} {yields} A{sub 1g} fluorescence quantum yield of benzene has been obtained for excitations from 250 to 150 nm in the solvents n-hexane, isooctane, n-perfluorohexane, n-pentane, cyclohexane, and cis-decalin. In n-hexane and isooctane, measurements have been made over a range of benzene concentrations from 0.11{sub 2} to 11.2 M (the neat liquid). In dilute solutions, the sudden losses in fluorescence as the excitation wavelength sweeps from the first into the second absorption system and then again as the excitation wavelength sweeps from the second into the third absorption system are correlated with the behavior of benzene vapor in the region of channel three. Increasing the benzene concentration causes abatements in the rate of loss of fluorescence with decreasing excitation wavelength in the regions of the second and third absorption systems and, above 2 M, causes a reversal of this rate so as to cause a recovery of the fluorescence in the region of the third absorption system. These changes are correlated with the effects of benzene concentration on the electronic absorption spectrum and with reported effects of clustering on the multiphoton photoionization efficiency. 59 refs., 13 figs.

  1. Search for 2 ν β β decay of 136Xe to the 01+ excited state of 136Ba with the EXO-200 liquid xenon detector

    NASA Astrophysics Data System (ADS)

    Albert, J. B.; Auty, D. J.; Barbeau, P. S.; Beck, D.; Belov, V.; Breidenbach, M.; Brunner, T.; Burenkov, A.; Cao, G. F.; Chambers, C.; Chaves, J.; Cleveland, B.; Coon, M.; Craycraft, A.; Daniels, T.; Danilov, M.; Daugherty, S. J.; Davis, J.; Delaquis, S.; Der Mesrobian-Kabakian, A.; DeVoe, R.; Didberidze, T.; Dilling, J.; Dolgolenko, A.; Dolinski, M. J.; Dunford, M.; Fairbank, W.; Farine, J.; Feldmeier, W.; Feyzbakhsh, S.; Fierlinger, P.; Fudenberg, D.; Gornea, R.; Graham, K.; Gratta, G.; Hall, C.; Hughes, M.; Jewell, M. J.; Johnson, A.; Johnson, T. N.; Johnston, S.; Karelin, A.; Kaufman, L. J.; Killick, R.; King, J.; Koffas, T.; Kravitz, S.; Krücken, R.; Kuchenkov, A.; Kumar, K. S.; Leonard, D. S.; Licciardi, C.; Lin, Y. H.; Ling, J.; MacLellan, R.; Marino, M. G.; Mong, B.; Moore, D.; Njoya, O.; Nelson, R.; Odian, A.; Ostrovskiy, I.; Piepke, A.; Pocar, A.; Prescott, C. Y.; Retière, F.; Rowson, P. C.; Russell, J. J.; Schubert, A.; Sinclair, D.; Smith, E.; Stekhanov, V.; Tarka, M.; Tolba, T.; Tsang, R.; Twelker, K.; Vogel, P.; Vuilleumier, J.-L.; Waite, A.; Walton, J.; Walton, T.; Weber, M.; Wen, L. J.; Wichoski, U.; Winick, T. A.; Wood, J.; Xu, Q. Y.; Yang, L.; Yen, Y.-R.; Zeldovich, O. Ya.; EXO-200 Collaboration

    2016-03-01

    EXO-200 is a single phase liquid xenon detector designed to search for neutrinoless β β decay of 136Xe to the ground state of 136Ba. We report here on a search for the two-neutrino β β decay of 136Xe to the first 0+ excited state, 01+, of 136Ba based on a 100 kg yr exposure of 136Xe. Using a specialized analysis employing a machine learning algorithm, we obtain a 90% CL half-life sensitivity of 1.7 ×1024 yr. We find no statistically significant evidence for the 2 ν β β decay to the excited state resulting in a lower limit of T1/2 2 ν (0+→01+) > 6.9 ×1023 yr at 90% CL. This observed limit is consistent with the estimated half-life of 2.5 ×1025 yr.

  2. Fluorescence resonance energy transfer in microemulsions composed of tripled-chain surface active ionic liquids, RTILs, and biological solvent: an excitation wavelength dependence study.

    PubMed

    Banerjee, Chiranjib; Kundu, Niloy; Ghosh, Surajit; Mandal, Sarthak; Kuchlyan, Jagannath; Sarkar, Nilmoni

    2013-08-15

    In this article we have reported the fluorescence resonance energy transfer (FRET) study in our earlier characterized surface active ionic liquids (SAILs)-containing microemulsion, i.e., N-methyl-N-propylpyrrolidinium bis(trifluoromethanesulfonyl)imide ([P13][Tf2N])/[CTA][AOT]/isopropyl myristate ([IPM]) and N,N,N-trimethyl-N-propylammonium bis(trifluoromethanesulfonyl)imide ([N3111][Tf2N])/[CTA][AOT]/[IPM] microemulsions (Banerjee, C.; Mandal, S.; Ghosh, S.; Kuchlyan, J.; Kundu, N.; Sarkar, N. J. Phys. Chem. B 2013, 117, 3927-3934). The occurrence of effective FRET from the donor, coumarin-153 (C-153) to the acceptor rhodamine 6G (R6G) is evident from the decrease in the steady state fluorescence intensity of the donor with addition of acceptor and subsequent increase in the fluorescence intensity of the acceptor in the presence of donor. The excitation wavelength dependent FRET from C-153 to R6G has also been performed to assess the dynamic heterogeneity of these confined systems. In time-resolved experiments, the significant rise time of the acceptor in the presence of the donor further confirms the occurrence of FRET. The multiple donor-acceptor (D-A) distances, for various microemulsions, obtained from the rise times of the acceptor emission in the presence of a donor can be rationalized from the varying distribution of the donor, C-153, in the different regions of the microemulsion. Time-resolved measurement reveals that with increasing excitation wavelength from 408 to 440 nm, the contribution of the faster rise component of FRET increases significantly due to the close proximity of the C-153 and R6G in the polar region of the microemulsion where occurrence of FRET is very high. Moreover, we have also studied the FRET with variation of R (R = [room temperature ionic liquids (RTILs)]/[surfactant]) and shown that the effect of excitation wavelength on FRET is similar irrespective of R values.

  3. Formation of excited states of N,N,N',N'-tetramethyl-p-phenylenediamine in irradiated nonpolar liquids. [Electron beams

    SciTech Connect

    Choi, H.T.; Tweeten, D.W.; Lipsky, S.

    1984-11-22

    The yield of N,N,N',N'-tetramethyl-p-phenylenediamine (TMPD) excited states, G/sub s/, has been obtained in irradiated tetramethylsilane, isooctane, cyclopentane, n-hexane, and cyclohexane as a function of TMPD concentration, c, over the range c = 0.5 x 10/sup -3/-50 x 10/sup -3/ M. In tetramethylsilane and isooctane, G/sub s/ is found to be linear on c as would be expected on the basis of a nondiffusional transfer of the solvent ion positive charge to TMPD followed by recombination of TMPD/sup +/ with the geminate electron. In cyclopentane, n-hexane, and cyclohexane, G/sub s/ becomes increasingly concave downward in its depedence on c. This concavity is attributed to an increasing contribution to G/sub s/ from excited states of the solvent that nonradiatively transfer their energy to TMPD. Optical excitation of cyclohexane at 147 nm and measurement of the quenching of its fluorescence by TMPD confirm this view.

  4. An apparatus for pulsed ESR and DNP experiments using optically excited triplet states down to liquid helium temperatures

    NASA Astrophysics Data System (ADS)

    Eichhorn, T. R.; Haag, M.; van den Brandt, B.; Hautle, P.; Wenckebach, W. Th.; Jannin, S.; van der Klink, J. J.; Comment, A.

    2013-09-01

    In standard Dynamic Nuclear Polarization (DNP) electron spins are polarized at low temperatures in a strong magnetic field and this polarization is transferred to the nuclear spins by means of a microwave field. To obtain high nuclear polarizations cryogenic equipment reaching temperatures of 1 K or below and superconducting magnets delivering several Tesla are required. This equipment strongly limits applications in nuclear and particle physics where beams of particles interact with the polarized nuclei, as well as in neutron scattering science. The problem can be solved using short-lived optically excited triplet states delivering the electron spin. The spin is polarized in the optical excitation process and both the cryogenic equipment and magnet can be simplified significantly. A versatile apparatus is described that allows to perform pulsed dynamic nuclear polarization experiments at X-band using short-lived optically excited triplet sates. The efficient 4He flow cryostat that cools the sample to temperatures between 4 K and 300 K has an optical access with a coupling stage for a fiber transporting the light from a dedicated laser system. It is further designed to be operated on a neutron beam. A combined pulse ESR/DNP spectrometer has been developed to observe and characterize the triplet states and to perform pulse DNP experiments. The ESR probe is based on a dielectric ring resonator of 7 mm inner diameter that can accommodate cubic samples of 5 mm length needed for neutron experiments. NMR measurements can be performed during DNP with a coil integrated in the cavity. With the presented apparatus a proton polarization of 0.5 has been achieved at 0.3 T.

  5. An apparatus for pulsed ESR and DNP experiments using optically excited triplet states down to liquid helium temperatures.

    PubMed

    Eichhorn, T R; Haag, M; van den Brandt, B; Hautle, P; Wenckebach, W Th; Jannin, S; van der Klink, J J; Comment, A

    2013-09-01

    In standard Dynamic Nuclear Polarization (DNP) electron spins are polarized at low temperatures in a strong magnetic field and this polarization is transferred to the nuclear spins by means of a microwave field. To obtain high nuclear polarizations cryogenic equipment reaching temperatures of 1 K or below and superconducting magnets delivering several Tesla are required. This equipment strongly limits applications in nuclear and particle physics where beams of particles interact with the polarized nuclei, as well as in neutron scattering science. The problem can be solved using short-lived optically excited triplet states delivering the electron spin. The spin is polarized in the optical excitation process and both the cryogenic equipment and magnet can be simplified significantly. A versatile apparatus is described that allows to perform pulsed dynamic nuclear polarization experiments at X-band using short-lived optically excited triplet sates. The efficient (4)He flow cryostat that cools the sample to temperatures between 4 K and 300 K has an optical access with a coupling stage for a fiber transporting the light from a dedicated laser system. It is further designed to be operated on a neutron beam. A combined pulse ESR/DNP spectrometer has been developed to observe and characterize the triplet states and to perform pulse DNP experiments. The ESR probe is based on a dielectric ring resonator of 7 mm inner diameter that can accommodate cubic samples of 5mm length needed for neutron experiments. NMR measurements can be performed during DNP with a coil integrated in the cavity. With the presented apparatus a proton polarization of 0.5 has been achieved at 0.3 T.

  6. Mobile impurities in ferromagnetic liquids

    NASA Astrophysics Data System (ADS)

    Kantian, Adrian; Schollwoeck, Ulrich; Giamarchi, Thierry

    2011-03-01

    Recent work has shown that mobile impurities in one dimensional interacting systems may exhibit behaviour that differs strongly from that predicted by standard Tomonaga-Luttinger liquid theory, with the appearance of power-law divergences in the spectral function signifying sublinear diffusion of the impurity. Using time-dependent matrix product states, we investigate a range of cases of mobile impurities in systems beyond the analytically accessible examples to assess the existence of a new universality class of low-energy physics in one-dimensional systems. Correspondence: Adrian.Kantian@unige.ch This work was supported in part by the Swiss SNF under MaNEP and division II.

  7. Search for 2νββ decay of Xe136 to the 01+ excited state of Ba136 with the EXO-200 liquid xenon detector

    DOE PAGES

    Albert, J. B.; Auty, D. J.; Barbeau, P. S.; Beck, D.; Belov, V.; Breidenbach, M.; Brunner, T.; Burenkov, A.; Cao, G. F.; Chambers, C.; et al

    2016-03-08

    EXO-200 is a single phase liquid xenon detector designed to search for neutrinoless ββ decay of 136Xe to the ground state of 136Ba. We report here on a search for the two-neutrino ββ decay of 136Xe to the first 0+ excited state, 0+1, of Ba136 based on a 100 kg yr exposure of 136Xe. Using a specialized analysis employing a machine learning algorithm, we obtain a 90% CL half-life sensitivity of 1.7×1024 yr. We find no statistically significant evidence for the 2νββ decay to the excited state resulting in a lower limit of T2ν1/2 (0+ → 0+1) > 6.9 ×1023more » yr at 90% CL. In conclusion, this observed limit is consistent with the estimated half-life of 2.5×1025 yr.« less

  8. Collective excitations of strongly coupled bilayer charged Bose liquids in the third-frequency-moment sum rule

    NASA Astrophysics Data System (ADS)

    Tas, Murat; Tanatar, B.

    2008-09-01

    We calculate the collective excitation modes of strongly coupled bilayer charged Bose systems. We employ the dielectric matrix formulation to study the correlation effects within the random-phase approximation (RPA), the self consistent field approximation Singwi, Tosi, Land, and Sjölander (STLS), and the quasilocalized charge approximation (QLCA), which satisfies the third-frequency-moment (⟨ω3⟩) sum rule. We find that the QLCA predicts a long-wavelength correlation-induced energy gap in the out-of-phase plasmon mode, similar to the situation in electronic bilayer systems. The energy gap and the plasmon density of states are studied as a function of interlayer separation and coupling parameter rs . The results should be helpful for experimental investigations.

  9. Optical and application study of gas-liquid discharge excited by bipolar nanosecond pulse in atmospheric air

    NASA Astrophysics Data System (ADS)

    Wang, Sen; Wang, Wen-chun; Yang, De-zheng; Liu, Zhi-jie; Zhang, Shuai

    2014-10-01

    In this study, a bipolar nanosecond pulse with 20 ns rising time is employed to generate air gas-liquid diffuse discharge plasma with room gas temperature in quartz tube at atmospheric pressure. The image of the discharge and optical emission spectra of active species in the plasma are recorded. The plasma gas temperature is determined to be approximately 390 K by compared the experimental spectra with the simulated spectra, which is slightly higher than the room temperature. The result indicated that the gas temperature rises gradually with pulse peak voltage increasing, while decreases slightly with the electrode gap distance increasing. As an important application, bipolar nanosecond pulse discharge is used to sterilize the common microorganisms (Actinomycetes, Candida albicans and Escherichia coli) existing in drinking water, which performs high sterilization efficiency.

  10. Optical and application study of gas-liquid discharge excited by bipolar nanosecond pulse in atmospheric air.

    PubMed

    Wang, Sen; Wang, Wen-chun; Yang, De-zheng; Liu, Zhi-jie; Zhang, Shuai

    2014-10-15

    In this study, a bipolar nanosecond pulse with 20ns rising time is employed to generate air gas-liquid diffuse discharge plasma with room gas temperature in quartz tube at atmospheric pressure. The image of the discharge and optical emission spectra of active species in the plasma are recorded. The plasma gas temperature is determined to be approximately 390K by compared the experimental spectra with the simulated spectra, which is slightly higher than the room temperature. The result indicated that the gas temperature rises gradually with pulse peak voltage increasing, while decreases slightly with the electrode gap distance increasing. As an important application, bipolar nanosecond pulse discharge is used to sterilize the common microorganisms (Actinomycetes, Candida albicans and Escherichia coli) existing in drinking water, which performs high sterilization efficiency.

  11. Holographic quantum liquids in 1+1 dimensions

    NASA Astrophysics Data System (ADS)

    Hung, Ling-Yan; Sinha, Aninda

    2010-01-01

    In this paper we initiate the study of holographic quantum liquids in 1+1 dimensions. Since the Landau Fermi liquid theory breaks down in 1+1 dimensions, it is of interest to see what holographic methods have to say about similar models. For theories with a gapless branch, the Luttinger conjecture states that there is an effective description of the physics in terms of a Luttinger liquid which is specified by two parameters. The theory we consider is the defect CFT arising due to a probe D3 brane in the AdS Schwarzschild planar black hole background. We turn on a fundamental string density on the worldvolume. Unlike higher dimensional defects, a persistent dissipationless zero sound mode is found. The thermodynamic aspects of these models are considered carefully and certain subtleties with boundary terms are explained which are unique to 1+1 dimensions. Spectral functions of bosonic and fermionic fluctuations are also considered and quasinormal modes are analysed. A prescription is given to compute spectral functions when there is mixing due to the worldvolume gauge field. We comment on the Luttinger conjecture in the light of our findings.

  12. The Kohn-Luttinger mechanism and phase diagram of the superconducting state in the Shubin-Vonsovsky model

    SciTech Connect

    Kagan, M. Yu.; Val'kov, V. V.; Mitskan, V. A.; Korovuskin, M. M.

    2013-10-15

    Using the Shubin-Vonsovsky model in the weak-coupling regime W > U > V (W is the bandwidth, U is the Hubbard onsite repulsion, and V is the Coulomb interaction at neighboring sites) based on the Kohn-Luttinger mechanism, we determined the regions of the existence of the superconducting phases with the d{sub xy}, p, s, and d{sub x{sup 2}-y{sup 2}} symmetry types of the order parameter. It is shown that the effective interaction in the Cooper channel considerably depends not only on single-site but also on intersite Coulomb correlations. This is demonstrated by the example of the qualitative change and complication of the phase diagram of the superconducting state. The superconducting (SC) phase induction mechanism is determined taking into account polarization contributions in the second-order perturbation theory in the Coulomb interaction. The results obtained for the angular dependence of the superconducting gap in different channels are compared with angule-resolved photoemission spectroscopy (ARPES) results. The influence of long-range hops in the phase diagram and critical superconducting transition temperature in different channels is analyzed. The conditions for the appearance of the Kohn-Luttinger superconductivity with the d{sub x{sup 2}-y{sup 2}} symmetry and high critical temperatures T{sub c} {approx} 100 K near the half-filling are determined.

  13. Graphene quantum dots from graphite by liquid exfoliation showing excitation-independent emission, fluorescence upconversion and delayed fluorescence.

    PubMed

    Sarkar, Suprabhat; Gandla, Dayakar; Venkatesh, Yeduru; Bangal, Prakriti Ranjan; Ghosh, Sutapa; Yang, Yang; Misra, Sunil

    2016-08-21

    Facile synthesis of 2-10 nm-sized graphene quantum dots (GQDs) from graphite powder by organic solvent-assisted liquid exfoliation using a sonochemical method is reported in this study. Synthesized GQDs are well dispersed in organic solvents like ethyl acetoacetate (EAA), dimethyl formamide (DMF) and also in water. MALDI-TOF mass spectrometry reveals its selective mass fragmentation. Detailed characterizations by various techniques like X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), X-ray photoelectron spectroscopy (XPS), Raman spectroscopy and high resolution transmission electron microscopy (HRTEM) confirm the formation of disordered, functional GQDs. Density functional theory (DFT) calculation confirms HOMO-LUMO energy gap variation with changing size and functionalities. Photoluminescence (PL) properties of as-prepared GQDs were studied in detail. The ensemble studies of GQDs showed excellent photoluminescence properties comprising normal and upconverted fluorescence, delayed fluorescence and room-temperature phosphorescence. PL decay dynamics of GQDs has been explored using time-correlated single-photon technique (TCSPC) as well as femtosecond fluorescence upconversion technique. In vitro cytotoxicity study reveals its biocompatibility and high cell viability (>91%) even at high concentration (400 μg mL(-1)) of GQDs in Chinese Hamster Ovary (CHO) cells. PMID:27302411

  14. Clues and criteria for designing a Kitaev spin liquid revealed by thermal and spin excitations of the honeycomb iridate Na2IrO3

    NASA Astrophysics Data System (ADS)

    Yamaji, Youhei; Suzuki, Takafumi; Yamada, Takuto; Suga, Sei-ichiro; Kawashima, Naoki; Imada, Masatoshi

    2016-05-01

    Contrary to the original expectation, Na2IrO3 is not a Kitaev's quantum spin liquid (QSL) but shows a zigzag-type antiferromagnetic order in experiments. Here, we propose experimental clues and criteria to measure how a material in hand is close to the Kitaev's QSL state. For this purpose, we systematically study thermal and spin excitations of a generalized Kitaev-Heisenberg model studied by Chaloupka et al., Phys. Rev. Lett. 110, 097204 (2013), 10.1103/PhysRevLett.110.097204 and an effective ab initio Hamiltonian for Na2IrO3 proposed by Yamaji et al., Phys. Rev. Lett. 113, 107201 (2014), 10.1103/PhysRevLett.113.107201, by employing a numerical diagonalization method. We reveal that closeness to the Kitaev's QSL is characterized by the following properties, besides trivial criteria such as reduction of magnetic ordered moments and Néel temperatures. (1) Two peaks in the temperature dependence of specific heat at Tℓ and Th caused by the fractionalization of spin to two types of Majorana fermions. (2) In between the double peak, a prominent plateau or shoulder pinned at R/2 ln2 in the temperature dependence of entropy, where R is the gas constant. (3) Failure of the linear spin wave approximation at the low-lying excitations of dynamical structure factors. (4) Small ratio Tℓ/Th close to or less than 0.03. According to the proposed criteria, Na2IrO3 is categorized to a compound close to the Kitaev's QSL, and is proven to be a promising candidate for the realization of the QSL if the relevant material parameters can further be tuned by making thin film of Na2IrO3 on various substrates or applying axial pressure perpendicular to the honeycomb networks of iridium ions. Applications of these characterization to (Na1-xLix) 2IrO3 and other related materials are also discussed.

  15. Flowing Liquid Anode Atmospheric Pressure Glow Discharge as an Excitation Source for Optical Emission Spectrometry with the Improved Detectability of Ag, Cd, Hg, Pb, Tl, and Zn.

    PubMed

    Greda, Krzysztof; Swiderski, Krzysztof; Jamroz, Piotr; Pohl, Pawel

    2016-09-01

    A novel atmospheric pressure glow discharge generated in contact with a flowing liquid anode (FLA-APGD) was developed as the efficient excitation source for the optical emission spectrometry (OES) detection. Differences in the appearance and the electrical characteristic of the FLA-APGD and a conventional system operated with a flowing liquid cathode (FLC-APGD) were studied in detail and discussed. Under the optimal operating conditions for the FLA-APGD, the emission from the analytes (Ag, Cd, Hg, Pb, Tl, and Zn) was from 20 to 120 times higher as compared to the FLC-APGD. Limits of detections (LODs) established with a novel FLA-APGD system were on average 20 times better than those obtained for the FLC-APGD. A further improvement of the LODs was achieved by reducing the background shift interferences and, as a result, the LODs for Ag, Cd, Hg, Pb, Tl, and Zn were 0.004, 0.040, 0.70, 1.7, 0.035, and 0.45 μg L(-1), respectively. The precision of the FLA-APGD-OES method was evaluated to be within 2-5% (as the relative standard deviation of the repeated measurements). The method found its application in the determination of the content of Ag, Cd, Hg, Pb, Tl, and Zn in a certified reference material (CRM) of Lobster hepatopancreas (TORT-2), four brass samples as well as mineral water and tea leaves samples spiked with the analytes. In the case of brass samples, a reference method, i.e., inductively coupled plasma optical emission spectrometry (ICP-OES) was used. A good agreement between the results obtained with FLA-APGD-OES and the certified values for the CRM TORT-2 as well as the reference values obtained with ICP-OES for the brass samples was revealed, indicating the good accuracy of the proposed method. The recoveries obtained for the spiked samples of mineral water and tea leaves were within the range of 97.5-102%. PMID:27476678

  16. Identifying a Bath-Induced Bose Liquid in Interacting Spin-Boson Models

    NASA Astrophysics Data System (ADS)

    Cai, Zi; Schollwöck, Ulrich; Pollet, Lode

    2014-12-01

    We study the ground state phase diagram of a one-dimensional hard-core bosonic model with nearest-neighbor interactions (X X Z model) where every site is coupled Ohmically to an independent but identical reservoir, hereby generalizing spin-boson models to interacting spin-boson systems. We show that a bath-induced Bose liquid phase can occur in the ground state phase diagram away from half filling. This phase is compressible, gapless, and conducting but not superfluid. At half filling, only a Luttinger liquid and a charge density wave are found. The phase transition between them is of Kosterlitz-Thouless type where the Luttinger parameter takes a nonuniversal value. The applied quantum Monte Carlo method can be used for all open bosonic and unfrustrated spin systems, regardless of their dimension, filling factor, and spectrum of the dissipation as long as the quantum system couples to the bath via the density operators.

  17. Identifying a bath-induced bose liquid in interacting spin-boson models.

    PubMed

    Cai, Zi; Schollwöck, Ulrich; Pollet, Lode

    2014-12-31

    We study the ground state phase diagram of a one-dimensional hard-core bosonic model with nearest-neighbor interactions (XXZ model) where every site is coupled Ohmically to an independent but identical reservoir, hereby generalizing spin-boson models to interacting spin-boson systems. We show that a bath-induced Bose liquid phase can occur in the ground state phase diagram away from half filling. This phase is compressible, gapless, and conducting but not superfluid. At half filling, only a Luttinger liquid and a charge density wave are found. The phase transition between them is of Kosterlitz-Thouless type where the Luttinger parameter takes a nonuniversal value. The applied quantum Monte Carlo method can be used for all open bosonic and unfrustrated spin systems, regardless of their dimension, filling factor, and spectrum of the dissipation as long as the quantum system couples to the bath via the density operators.

  18. Non-Fermi-liquid behavior in the fluctuating gap model: From the pole to a zero of the Green's function

    SciTech Connect

    Kuchinskii, E. Z.; Sadovskii, M. V.

    2006-09-15

    We analyze the non-Fermi-liquid (NFL) behavior of the fluctuating gap model (FGM) of pseudogap behavior in both one and two dimensions. A detailed discussion of quasiparticle renormalization (Z-factor) is given, demonstrating a kind of marginal Fermi-liquid or Luttinger-liquid behavior and topological stability of the bare Fermi surface (the Luttinger theorem). In the two-dimensional case, we discuss the effective picture of the Fermi surface destruction both in the hot spot model of dielectric (AFM, CDW) pseudogap fluctuations and for the qualitatively different case of superconducting d-wave fluctuations, reflecting the NFL spectral density behavior and similar to that observed in ARPES experiments on copper oxides.

  19. Towards an easy-to-use tuberculosis diagnosis through exhaled breath analysis: a liquid fluorimeter with an excitation at 265 nm

    NASA Astrophysics Data System (ADS)

    Hue, J.; Dupoy, M.; Vignoud, S.; Ricaud, J. L.; Tran-Thi, T.; Karpe, S.; Novelli-Rousseau, A.; Mallard, F.

    2013-03-01

    The struggle against tuberculosis is one of the World Health Organization priorities. Identifying in a short time, patients with active tuberculosis, would bring a tremendous improvement to the current situation. Recovering from this infectious and deadly disease (2 million of death per year) is possible with a correct diagnosis to give an appropriate treatment. Unfortunately, most common tuberculosis diagnoses have few drawbacks: - skin tests: not reliable at 100% and need an incubation of 2 days before the diagnosis, - blood tests: costly and sophisticated technology, - chest X-ray: the first step before the sputum tests used for a bacterial culture with a final diagnosis given within 2 weeks. A tuberculosis test based on exhaled breath analysis is a prospective and noninvasive solution, cheap and easy to use and to transport. This test lies on a fluoregenic detection of niacin, a well-known mycobacterium tuberculosis specific metabolite. In this paper, it is assumed that the selected probe is specific to niacin and that exhaled breath does not contain any interfering species. To address this problem, a fluorimeter is developed with a cheap and cooled CCD ( 2k$) as a sensor, to easily determine the suitable "fluorescent zone". In comparing aqueous solutions with and without niacin, 250 pM of niacin have been detected. With a commercial fluorimeter (Fluorolog from Horiba), only 200 nM of niacin are detected. The present detection remains 10 times above the estimated targeted value for a tuberculosis test. The excitation source is a LED, which typically emits 20 °W at 265 nm through an optical fiber. The emission signal is detected around 545 nm. A typical light exposure lasts 700 seconds. Analysis of biomarkers with a liquid fluorimeter is generic and promising as health diagnosis.

  20. Mise en évidence d'états excités dans les spectres de photoionisation du cyclohexane et du diméthyl 2-2-butane liquides

    NASA Astrophysics Data System (ADS)

    Casanovas, J.; Guelfucci, J. P.; Caselles, O.

    1991-07-01

    Excited states are probably occurring, at an intermediate stage, in the VUV photoionization process of liquid hydrocarbons, as suggested by a Stern-Volmer behaviour when interacting with electron quenchers. They are here detected in the VUV photoionization spectrum of cyclohexane and dimethyl-2-2-butane in liquid phase. Some of the discernable peaks can be assigned as valence and Rydberg states, yet observed in gas phase. Supplementary peaks are observed, the existence of which is to be interpretated. L'existence d'états excités dans le processus de photoionisation VUV des hydrocarbures en phase liquide - précédemment suggérée par l'observation de la loi de Stern-Volmer lors de l'interaction avec des capteurs d'électrons - est ici détectée en traçant le spectre de photoionisation VUV du cyclohexane et du diméthyl-2-2-butane purs en phase liquide. Certains des pics observés coïncident avec les états de valence et de Rydberg de ces mêmes corps en phase gaz. Il apparaît des pics supplémentaires dont la nature doit être précisée.

  1. Dynamical functions of a 1D correlated quantum liquid

    NASA Astrophysics Data System (ADS)

    Carmelo, J. M. P.; Bozi, D.; Penc, K.

    2008-10-01

    The dynamical correlation functions in one-dimensional electronic systems show power-law behaviour at low energies and momenta close to integer multiples of the charge and spin Fermi momenta. These systems are usually referred to as Tomonaga-Luttinger liquids. However, near well defined lines of the (k,ω) plane the power-law behaviour extends beyond the low-energy cases mentioned above, and also appears at higher energies, leading to singular features in the photoemission spectra and other dynamical correlation functions. The general spectral-function expressions derived in this paper were used in recent theoretical studies of the finite-energy singular features in photoemission of the organic compound tetrathiafulvalene-tetracyanoquinodimethane (TTF-TCNQ) metallic phase. They are based on a so-called pseudofermion dynamical theory (PDT), which allows us to systematically enumerate and describe the excitations in the Hubbard model starting from the Bethe ansatz, as well as to calculate the charge and spin object phase shifts appearing as exponents of the power laws. In particular, we concentrate on the spin-density m\\rightarrow 0 limit and on effects in the vicinity of the singular border lines, as well as close to half filling. Our studies take into account spectral contributions from types of microscopic processes that do not occur for finite values of the spin density. In addition, the specific processes involved in the spectral features of TTF-TCNQ are studied. Our results are useful for the further understanding of the unusual spectral properties observed in low-dimensional organic metals and also provide expressions for the one- and two-atom spectral functions of a correlated quantum system of ultracold fermionic atoms in a 1D optical lattice with on-site two-atom repulsion.

  2. Nonexistence of the Luttinger-Ward functional and misleading convergence of skeleton diagrammatic series for hubbard-like models.

    PubMed

    Kozik, Evgeny; Ferrero, Michel; Georges, Antoine

    2015-04-17

    The Luttinger-Ward functional Φ[G], which expresses the thermodynamic grand potential in terms of the interacting single-particle Green's function G, is found to be ill defined for fermionic models with the Hubbard on-site interaction. In particular, we show that the self-energy Σ[G]∝δΦ[G]/δG is not a single-valued functional of G: in addition to the physical solution for Σ[G], there exists at least one qualitatively distinct unphysical branch. This result is demonstrated for several models: the Hubbard atom, the Anderson impurity model, and the full two-dimensional Hubbard model. Despite this pathology, the skeleton Feynman diagrammatic series for Σ in terms of G is found to converge at least for moderately low temperatures. However, at strong interactions, its convergence is to the unphysical branch. This reveals a new scenario of breaking down of diagrammatic expansions. In contrast, the bare series in terms of the noninteracting Green's function G0 converges to the correct physical branch of Σ in all cases currently accessible by diagrammatic Monte Carlo calculations. In addition to their conceptual importance, these observations have important implications for techniques based on the explicit summation of the diagrammatic series. PMID:25933324

  3. Excited-State Tautomerization of 7-Azaindole in Nonpolar Solution: A Theoretical Study Based on Liquid-Phase Potential Surfaces of Mean Force.

    PubMed

    Fang, Hua; Kim, Yongho

    2013-08-13

    Excited state tautomerization of a 7-azaindole (7AI) complex with one methanol molecule in heptane was studied using variational transition state theory including multidimensional tunneling (VTST/MT) with the dielectric continuum model for the solvent effect. Electronic structures and energies for reactants and transition state (TS) in solution were computed at the complete active space self-consistent field (CASSCF) level with second-order multireference perturbation theory (MRPT2) to take into consideration of dynamic electron correlation. The polarizable continuum model using the integral equation formalism (IEFPCM) and the SMD model were used for the excited-state solvent effect. Excited-state surfaces of potential of the mean force in solution were generated for the first time at the MRPT2//SMD/CASSCF(10,9)/6-31G(d,p) level. The position of TS on the reaction coordinate substantially depended on the dynamic electron correlation. The two protons in the excited-state tautomerization were transferred in a concerted but asynchronous process. Calculated HH/DD kinetic isotope effect (KIE) and the ratio of Arrhenius pre-exponential factors, A(HH)/A(DD), agreed very well with the corresponding experimental values. The shape of the adiabatic energy surfaces in the excited-state strongly depended on the position of isotopes due to the asynchronicity of the reaction path, and the tunneling effect was essential for reproducing experimental KIEs. The pyrrolic proton moved a twice longer distance by tunneling than the hydroxyl proton in the most probable tunneling path at 292 K. This study strongly suggests that the mechanism of the excited-state double proton transfer in heptane is triggered by proton transfer from the pyrrolic nitrogen of 7AI to alcohol (protolytic pathway), rather than by proton transfer from alcohol to the pyridine nitrogen of 7AI (solvolytic pathway).

  4. Deuterated analogues as internal reference compounds for the direct determination of benzo(a)pyrene and perylene in liquid fuels by laser-excited Shpol'skii spectrometry

    SciTech Connect

    Yen Yang

    1981-11-01

    The polycyclic aromatic hydrocarbon (PAH) content of coal liquefaction products and other liquid fuels is usually assessed by measuring the benzo(a)pyrene content. In Shpol'skii effect spectrometry, PAHs and their deuterated analogues exhibit adequately resolved characteristic quasi-line spectra. The authors have used deuterated benzo(a)pyrene and perylene as externally added internal reference compounds to facilitate the direct determination of benzo(a)pyrene and perylene in liquid fuels.

  5. Synchrotron-radiation study of weak fluorescence from neat liquids of simple alkenes: Anomalous excitation spectra as evidence for wavelength-dependent photochemistry

    SciTech Connect

    Inoue, Yoshihisa; Daino, Yoshihiko; Tai, Akira; Hakushi, Tadao ); Okada, Tadashi )

    1989-07-19

    Fluorescence excitation spectra of trans-2-octene, trans-cyclooctene, 2-methyl-2-butene, and 2,3-dimethyl-2-butene were measured by using synchrotron radiation as a tunable light source in the vacuum UV and UV region. The wavelength dependence of the fluorescence yields provides direct evidence for the long-proposed assignment that the emissive state is the {pi},R(3s) Rydberg state, which in turn gives the carbene-derived photoproducts.

  6. Magnetostrictive resonance excitation

    DOEpatents

    Schwarz, Ricardo B.; Kuokkala, Veli-Tapani

    1992-01-01

    The resonance frequency spectrum of a magnetostrictive sample is remotely determined by exciting the magnetostrictive property with an oscillating magnetic field. The permeability of a magnetostrictive material and concomitant coupling with a detection coil varies with the strain in the material whereby resonance responses of the sample can be readily detected. A suitable sample may be a magnetostrictive material or some other material having at least one side coated with a magnetostrictive material. When the sample is a suitable shape, i.e., a cube, rectangular parallelepiped, solid sphere or spherical shell, the elastic moduli or the material can be analytically determined from the measured resonance frequency spectrum. No mechanical transducers are required and the sample excitation is obtained without contact with the sample, leading to highly reproducible results and a measurement capability over a wide temperature range, e.g. from liquid nitrogen temperature to the Curie temperature of the magnetostrictive material.

  7. Excited Delirium

    PubMed Central

    Takeuchi, Asia; Ahern, Terence L.; Henderson, Sean O.

    2011-01-01

    Excited (or agitated) delirium is characterized by agitation, aggression, acute distress and sudden death, often in the pre-hospital care setting. It is typically associated with the use of drugs that alter dopamine processing, hyperthermia, and, most notably, sometimes with death of the affected person in the custody of law enforcement. Subjects typically die from cardiopulmonary arrest, although the cause is debated. Unfortunately an adequate treatment plan has yet to be established, in part due to the fact that most patients die before hospital arrival. While there is still much to be discovered about the pathophysiology and treatment, it is hoped that this extensive review will provide both police and medical personnel with the information necessary to recognize and respond appropriately to excited delirium. PMID:21691475

  8. Excited baryons

    SciTech Connect

    Mukhopadhyay, N.C.

    1986-01-01

    The status of the theory of the low-energy approach to hadron structure is reviewed briefly by surveying a few relevant models. A few examples of tests needed to sort out the predictions of different models pertaining to the quark-gluon structure of hadrons are discussed, and given the resulting physics objectives, a few experimental options for excited baryon research at CFBAF are suggested. (LEW)

  9. Sexual excitement.

    PubMed

    Stoller, R J

    1976-08-01

    Sexual excitement depends on a scenario the person to be aroused has been writing since childhood. The story is an adventure, an autobiography disguised as fiction, in which the hero/heroine hides crucial intrapsychic conflicts, mysteries, screen memories of actual traumatic events and the resolution of these elements into a happy ending, best celebrated by orgasm. The function of the fantasy is to take these painful experiences and convert them to pleasure-triumph. In order to sharpen excitement-the vibration between the fear of original traumas repeating and the hope of a pleasurable conclusion this time-one introduces into the story elements of risk (approximations of the trauma) meant to prevent boredom and safety factors (sub-limnal signals to the storyteller that the risk are not truly dangerous). Sexual fantasy can be studied by means of a person's daydreams (including those chosen in magazines, books, plays, television, movies, and outright pornography), masturbatory behavior, object choice, foreplay, techniques of intercourse, or postcoital behavior. PMID:949223

  10. Sexual excitement.

    PubMed

    Stoller, R J

    1976-08-01

    Sexual excitement depends on a scenario the person to be aroused has been writing since childhood. The story is an adventure, an autobiography disguised as fiction, in which the hero/heroine hides crucial intrapsychic conflicts, mysteries, screen memories of actual traumatic events and the resolution of these elements into a happy ending, best celebrated by orgasm. The function of the fantasy is to take these painful experiences and convert them to pleasure-triumph. In order to sharpen excitement-the vibration between the fear of original traumas repeating and the hope of a pleasurable conclusion this time-one introduces into the story elements of risk (approximations of the trauma) meant to prevent boredom and safety factors (sub-limnal signals to the storyteller that the risk are not truly dangerous). Sexual fantasy can be studied by means of a person's daydreams (including those chosen in magazines, books, plays, television, movies, and outright pornography), masturbatory behavior, object choice, foreplay, techniques of intercourse, or postcoital behavior.

  11. Fermi Surface Evolution and Luttinger Theorem in NaxCoO2: A Systematic Photoemission Study

    SciTech Connect

    Yang, H. B.; Pan, Z. H.; Sekharan, A. K. P.; Sato, T.; Souma, S.; Takahashi, T.; Jin, Rongying; Sales, Brian C; Mandrus, David; Fedorov, A. V.; Wang, Z.; Ding, H.

    2005-01-01

    We report a systematic angle-resolved photoemission study on Na{sub x}CoO{sub 2} for a wide range of Na concentrations (0.3 {le} x {le} 0.72). In all the metallic samples at different x, we observed (i) only a single holelike Fermi surface centered around {Gamma} and (ii) its area changes with x according to the Luttinger theorem. We also observed a surface state that exhibits a larger Fermi surface area. The e{prime}{sub g} band and the associated small Fermi surface pockets near the K points predicted by band calculations are found to sink below the Fermi energy in a manner almost independent of the doping and temperature.

  12. White-light-exciting, layer-by-layer-assembled ZnCdHgSe quantum dots/polymerized ionic liquid hybrid film for highly sensitive photoelectrochemical immunosensing of neuron specific enolase.

    PubMed

    Yu, Xiangyang; Wang, Yanying; Chen, Xuemin; Wu, Kangbing; Chen, Danchao; Ma, Ming; Huang, Zhenjia; Wu, Wangze; Li, Chunya

    2015-04-21

    ZnCdHgSe quantum dots (QDs) functionalized with N-acetyl-l-cysteine were synthesized and characterized. Through layer-by-layer assembling, the ZnCdHgSe QDs was integrated with a polymerized 1-decyl-3-[3-pyrrole-1-yl-propyl]imidazolium tetrafluoroborate (PDPIT) ionic liquid film modified indium tin oxide (ITO) electrode to fabricated a photoelectrochemical interface for the immobilization of rabbit antihuman neuron specific enolase (anti-NSE). After being treated with glutaraldehyde vapor and bovine serum albumin successively, an anti-NSE/ZnCdHgSe QDs/PDPIT/ITO sensing platform was established. Simplely using a white-light LED as an excitation source, the immunoassay of neuron specific enolase (NSE) was achieved through monitoring the photocurrent variation. The polymerized ionic liquid film was demonstrated to be an important element to enhance the photocurrent response of ZnCdHgSe QDs. The anti-NSE/ZnCdHgSe QDs/PDPIT/ITO based immunosensor presents excellent performances in neuron specific enolase determination. The photocurrent variation before and after being interacted with NSE exhibits a good linear relationship with the logarithm of its concentration (log cNSE) in the range from 1.0 pg mL(-1) to 100 ng mL(-1). The limit of detection of this immunosensor is able to reach 0.2 pg mL(-1) (S/N = 3). The determination of NSE in clinical human sera was also demonstrated using anti-NSE/ZnCdHgSe QDs/PDPIT/ITO electrode. The results were found comparable with those obtained by using enzyme-linked immunosorbent assay method. PMID:25790014

  13. Determination of high-molecular weight polycyclic aromatic hydrocarbons in high performance liquid chromatography fractions of coal tar standard reference material 1597a via solid-phase nanoextraction and laser-excited time-resolved Shpol'skii spectroscopy.

    PubMed

    Wilson, Walter B; Alfarhani, Bassam; Moore, Anthony F T; Bisson, Cristina; Wise, Stephen A; Campiglia, Andres D

    2016-02-01

    This article presents an alternative approach for the analysis of high molecular weight - polycyclic aromatic hydrocarbons (HMW-PAHs) with molecular mass 302 Da in complex environmental samples. This is not a trivial task due to the large number of molecular mass 302 Da isomers with very similar chromatographic elution times and similar, possibly even virtually identical, mass fragmentation patterns. The method presented here is based on 4.2K laser-excited time-resolved Shpol'skii spectroscopy, a high resolution spectroscopic technique with the appropriate selectivity for the unambiguous determination of PAHs with the same molecular mass. The potential of this approach is demonstrated here with the analysis of a coal tar standard reference material (SRM) 1597a. Liquid chromatography fractions were submitted to the spectroscopic analysis of five targeted isomers, namely dibenzo[a,l]pyrene, dibenzo[a,e]pyrene, dibenzo[a,i]pyrene, naphtho[2,3-a]pyrene and dibenzo[a,h]pyrene. Prior to analyte determination, the liquid chromatographic fractions were pre-concentrated with gold nanoparticles. Complete analysis was possible with microliters of chromatographic fractions and organic solvents. The limits of detection varied from 0.05 (dibenzo[a,l]pyrene) to 0.24 µg L(-1) (dibenzo[a,e]pyrene). The excellent analytical figures of merit associated to its non-destructive nature, which provides ample opportunity for further analysis with other instrumental methods, makes this approach an attractive alternative for the determination of PAH isomers in complex environmental samples.

  14. RESONANT CAVITY EXCITATION SYSTEM

    DOEpatents

    Baker, W.R.; Kerns, Q.A.; Riedel, J.

    1959-01-13

    An apparatus is presented for exciting a cavity resonator with a minimum of difficulty and, more specifically describes a sub-exciter and an amplifier type pre-exciter for the high-frequency cxcitation of large cavities. Instead of applying full voltage to the main oscillator, a sub-excitation voltage is initially used to establish a base level of oscillation in the cavity. A portion of the cavity encrgy is coupled to the input of the pre-exciter where it is amplified and fed back into the cavity when the pre-exciter is energized. After the voltage in the cavity resonator has reached maximum value under excitation by the pre-exciter, full voltage is applied to the oscillator and the pre-exciter is tunned off. The cavity is then excited to the maximum high voltage value of radio frequency by the oscillator.

  15. Acoustically excited heated jets. 1: Internal excitation

    NASA Technical Reports Server (NTRS)

    Lepicovsky, J.; Ahuja, K. K.; Brown, W. H.; Salikuddin, M.; Morris, P. J.

    1988-01-01

    The effects of relatively strong upstream acoustic excitation on the mixing of heated jets with the surrounding air are investigated. To determine the extent of the available information on experiments and theories dealing with acoustically excited heated jets, an extensive literature survey was carried out. The experimental program consisted of flow visualization and flowfield velocity and temperature measurements for a broad range of jet operating and flow excitation conditions. A 50.8-mm-diam nozzle was used for this purpose. Parallel to the experimental study, an existing theoretical model of excited jets was refined to include the region downstream of the jet potential core. Excellent agreement was found between theory and experiment in moderately heated jets. However, the theory has not yet been confirmed for highly heated jets. It was found that the sensitivity of heated jets to upstream acoustic excitation varies strongly with the jet operating conditions and that the threshold excitation level increases with increasing jet temperature. Furthermore, the preferential Strouhal number is found not to change significantly with a change of the jet operating conditions. Finally, the effects of the nozzle exit boundary layer thickness appear to be similar for both heated and unheated jets at low Mach numbers.

  16. Faraday Waves under Time-Reversed Excitation

    NASA Astrophysics Data System (ADS)

    Pietschmann, Dirk; Stannarius, Ralf; Wagner, Christian; John, Thomas

    2013-03-01

    Do parametrically driven systems distinguish periodic excitations that are time mirrors of each other? Faraday waves in a Newtonian fluid are studied under excitation with superimposed harmonic wave forms. We demonstrate that the threshold parameters for the stability of the ground state are insensitive to a time inversion of the driving function. This is a peculiarity of some dynamic systems. The Faraday system shares this property with standard electroconvection in nematic liquid crystals [J. Heuer , Phys. Rev. E 78, 036218 (2008)PLEEE81539-3755]. In general, time inversion of the excitation affects the asymptotic stability of a parametrically driven system, even when it is described by linear ordinary differential equations. Obviously, the observed symmetry has to be attributed to the particular structure of the underlying differential equation system. The pattern selection of the Faraday waves above threshold, on the other hand, discriminates between time-mirrored excitation functions.

  17. Non-Fermi-liquid and topological states with strong spin-orbit coupling.

    PubMed

    Moon, Eun-Gook; Xu, Cenke; Kim, Yong Baek; Balents, Leon

    2013-11-15

    We argue that a class of strongly spin-orbit-coupled materials, including some pyrochlore iridates and the inverted band gap semiconductor HgTe, may be described by a minimal model consisting of the Luttinger Hamiltonian supplemented by Coulomb interactions, a problem studied by Abrikosov and collaborators. It contains twofold degenerate conduction and valence bands touching quadratically at the zone center. Using modern renormalization group methods, we update and extend Abrikosov's classic work and show that interactions induce a quantum critical non-Fermi-liquid phase, stable provided time-reversal and cubic symmetries are maintained. We determine the universal power-law exponents describing various observables in this Luttinger-Abrikosov-Beneslavskii state, which include conductivity, specific heat, nonlinear susceptibility, and the magnetic Gruneisen number. Furthermore, we determine the phase diagram in the presence of cubic and/or time-reversal symmetry breaking perturbations, which includes a topological insulator and Weyl semimetal phases. Many of these phases possess an extraordinarily large anomalous Hall effect, with the Hall conductivity scaling sublinearly with magnetization σ(xy)∼M0.51.

  18. PREFACE: Functionalized Liquid Liquid Interfaces

    NASA Astrophysics Data System (ADS)

    Girault, Hubert; Kornyshev, Alexei A.; Monroe, Charles W.; Urbakh, Michael

    2007-09-01

    optical study. Film formation goes a step beyond adsorption; some surfactants form monolayers or multilayers at the interface. A polymer microfilm or a polymer-particle matrix can be synthesized at the liquid-liquid boundary. Such films exhibit unique adsorption and ion-intercalation properties of their own. Electrowetting refers broadly to the phenomenon in which an applied voltage modulates the shape of a liquid-liquid interface, essentially by altering the surface tension. Electric fields can be used to induce droplets on solid substrates to change shape, or to affect the structure of liquid-liquid emulsions. Various chemical reactions can be performed at the liquid-liquid boundary. Liquid-liquid microelectrodes allow detailed study of ion-transfer kinetics at the interface. Photochemical processes can also be used to control the conformations of molecules adsorbed at the interface. But how much precise control do we actually have on the state of the interfacial region? Several contributions to this issue address a system which has been studied for decades in electrochemistry, but remains essentially unfamilar to physicists. This is the interface between two immiscible electrolytic solutions (ITIES), a progressing interdisciplinary field in which condensed-matter physics and physical chemistry meet molecular electrochemistry. Why is it so exciting? The reason is simple. The ITIES is chargeable: when positioned between two electrodes it can be polarized, and back- to-back electrical double layers form on both sides of the liquid-liquid interface. Importantly, the term immiscible refers not only to oil and water but also to the electrolytes. Inorganic electrolytes, such as alkali halides, tend to stay in water, whereas organic electrolytes, such as tetrabutylammonium tetraphenylborate, stay in oil. This behaviour arises because energies of the order of 0.2-0.3 eV are needed to drive ions across the interface. As long as these free energies of transfer are not exceeded by

  19. Reprint of : Regular and singular Fermi liquid in triple quantum dots: Coherent transport studies

    NASA Astrophysics Data System (ADS)

    Tooski, S. B.; Ramšak, A.; Bułka, B. R.

    2016-08-01

    A system of three coupled quantum dots in a triangular geometry (TQD) with electron-electron interaction and symmetrically coupled to two leads is analyzed with respect to the electron transport by means of the numerical renormalization group. Varying gate potentials this system exhibits extremely rich range of regimes with different many-electron states with various local spin orderings. It is demonstrated how the Luttinger phase changes in a controlled manner which then via the Friedel sum rule formula exactly reproduces the conductance through the TQD system. The analysis of the uncoupled TQD molecule from the leads gives a reliable qualitative understanding of various relevant regimes and an insight into the phase diagram with the regular Fermi liquid and singular-Fermi liquid phases.

  20. A mixed quantum-classical molecular dynamics study of anti-tetrol and syn-tetrol dissolved in liquid chloroform II: infrared emission spectra, vibrational excited-state lifetimes, and nonequilibrium hydrogen-bond dynamics.

    PubMed

    Kwac, Kijeong; Geva, Eitan

    2013-11-21

    The effect of vibrational excitation and relaxation of the hydroxyl stretch on the hydrogen-bond structure and dynamics of stereoselectively synthesized syn-tetrol and anti-tetrol dissolved in deuterated chloroform are investigated via a mixed quantum-classical molecular dynamics simulation. Emphasis is placed on the changes in hydrogen-bond structure upon photoexcitation and the nonequilibrium hydrogen-bond dynamics that follows the subsequent relaxation from the excited to the ground vibrational state. The propensity to form hydrogen bonds is shown to increase upon photoexcitation of the hydroxyl stretch, thereby leading to a sizable red-shift of the infrared emission spectra relative to the corresponding absorption spectra. The vibrational excited state lifetimes are calculated within the framework of Fermi's golden rule and the harmonic-Schofield quantum correction factor, and found to be sensitive reporters of the underlying hydrogen-bond structure. The energy released during the relaxation from the excited to the ground state is shown to break hydrogen bonds involving the relaxing hydroxyl. The spectral signature of this nonequilibrium relaxation process is analyzed in detail.

  1. Liquid White Enamel.

    ERIC Educational Resources Information Center

    Widmar, Marge

    1985-01-01

    A secondary teacher describes how she has her students use liquid white enamel. With the enameling process, students can create lasting, exciting artwork. They can exercise an understanding of design and color while learning the value of careful, sustained craft skills. (RM)

  2. 8. POWERHOUSE INTERIOR SHOWING EXCITER No. 1 IN FOREGROUND, EXCITER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    8. POWERHOUSE INTERIOR SHOWING EXCITER No. 1 IN FOREGROUND, EXCITER No. 2., AND GENERATOR UNITS BEHIND EXCITER No. 2 IN BACKGROUND. EXCITER No. 1 GENERATOR HAS A COVER OVER TOP HALF OF COMMUTATOR ELEMENT. VIEW TO NORTHWEST. - Rush Creek Hydroelectric System, Powerhouse Exciters, Rush Creek, June Lake, Mono County, CA

  3. 16. EXCITERS, AND SYNCHROSCOPE GAUGE ON WALL. ACTIVE ELECTRIC EXCITER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    16. EXCITERS, AND SYNCHROSCOPE GAUGE ON WALL. ACTIVE ELECTRIC EXCITER AT REAR; UNUSED WATER-DRIVEN EXCITER IN FOREGROUND. VIEW TO SOUTH-SOUTHWEST. - Santa Ana River Hydroelectric System, SAR-2 Powerhouse, Redlands, San Bernardino County, CA

  4. Holographic Quantum Liquid

    SciTech Connect

    Karch, A.; Son, D. T.; Starinets, A. O.

    2009-02-06

    Quantum liquids are characterized by the distinctive properties such as the low-temperature behavior of heat capacity and the spectrum of low-energy quasiparticle excitations. In particular, at low temperature, Fermi liquids exhibit the zero sound, predicted by Landau in 1957 and subsequently observed in liquid He-3. In this Letter, we ask whether such characteristic behavior is present in theories with a holographically dual description. We consider a class of gauge theories with fundamental matter fields whose holographic dual in the appropriate limit is given in terms of the Dirac-Born-Infeld action in anti-de Sitter space. We find that these systems also exhibit a sound mode at zero temperature despite having a non-Fermi-liquid behavior of the specific heat. These properties suggest that holography identifies a new type of quantum liquid which potentially could be experimentally realized in strongly correlated systems.

  5. BROADBAND EXCITATION IN NUCLEAR MAGNETIC RESONANCE

    SciTech Connect

    Tycko, R.

    1984-10-01

    Theoretical methods for designing sequences of radio frequency (rf) radiation pulses for broadband excitation of spin systems in nuclear magnetic resonance (NMR) are described. The sequences excite spins uniformly over large ranges of resonant frequencies arising from static magnetic field inhomogeneity, chemical shift differences, or spin couplings, or over large ranges of rf field amplitudes. Specific sequences for creating a population inversion or transverse magnetization are derived and demonstrated experimentally in liquid and solid state NMR. One approach to broadband excitation is based on principles of coherent averaging theory. A general formalism for deriving pulse sequences is given, along with computational methods for specific cases. This approach leads to sequences that produce strictly constant transformations of a spin system. The importance of this feature in NMR applications is discussed. A second approach to broadband excitation makes use of iterative schemes, i.e. sets of operations that are applied repetitively to a given initial pulse sequences, generating a series of increasingly complex sequences with increasingly desirable properties. A general mathematical framework for analyzing iterative schemes is developed. An iterative scheme is treated as a function that acts on a space of operators corresponding to the transformations produced by all possible pulse sequences. The fixed points of the function and the stability of the fixed points are shown to determine the essential behavior of the scheme. Iterative schemes for broadband population inversion are treated in detail. Algebraic and numerical methods for performing the mathematical analysis are presented. Two additional topics are treated. The first is the construction of sequences for uniform excitation of double-quantum coherence and for uniform polarization transfer over a range of spin couplings. Double-quantum excitation sequences are demonstrated in a liquid crystal system. The

  6. The Prediction of a Gapless Topological ``Haldane Liquid'' Phase in a One-Dimensional Cold Polar Molecular Lattice

    NASA Astrophysics Data System (ADS)

    Kestner, Jason; Wang, Bin; Sau, Jay; Das Sarma, Sankar

    2011-03-01

    We show that ultracold two-component fermionic dipolar gases in an optical lattice with strong two-body on-site loss can be used to realize a tunable effective spin-one model. Fermion number conservation provides an unusual constraint that ∑ i (Siz) 2 is conserved, leading to a novel topological liquid phase in one dimension which can be thought of as the gapless analog of the Haldane gapped phase of a spin- one Heisenberg chain. The properties of this phase are calculated numerically via the infinite time-evolving block decimation method and analytically via a mapping to a one-mode Luttinger liquid with hidden spin information. Work supported by AFOSR-MURI, DARPA-QUEST, ARO-DARPA-OLE, and CNAM.

  7. Collective excitations on a surface of topological insulator

    PubMed Central

    2012-01-01

    We study collective excitations in a helical electron liquid on a surface of three-dimensional topological insulator. Electron in helical liquid obeys Dirac-like equation for massless particles and direction of its spin is strictly determined by its momentum. Due to this spin-momentum locking, collective excitations in the system manifest themselves as coupled charge- and spin-density waves. We develop quantum field-theoretical description of spin-plasmons in helical liquid and study their properties and internal structure. Value of spin polarization arising in the system with excited spin-plasmons is calculated. We also consider the scattering of spin-plasmons on magnetic and nonmagnetic impurities and external potentials, and show that the scattering occurs mainly into two side lobes. Analogies with Dirac electron gas in graphene are discussed. PACS: 73.20.Mf; 73.22.Lp; 75.25.Dk. PMID:22376744

  8. Excitation Methods for Bridge Structures

    SciTech Connect

    Farrar, C.R.; Duffy, T.A.; Cornwell, P.J.; Doebling, S.W.

    1999-02-08

    This paper summarizes the various methods that have been used to excited bridge structures during dynamic testing. The excitation methods fall into the general categories of ambient excitation methods and measured-input excitation methods. During ambient excitation the input to the bridge is not directly measured. In contrast, as the category label implies, measured-input excitations are usually applied at a single location where the force input to the structure can be monitored. Issues associated with using these various types of measurements are discussed along with a general description of the various excitation methods.

  9. Decoherence at constant excitation

    NASA Astrophysics Data System (ADS)

    Torres, J. M.; Sadurní, E.; Seligman, T. H.

    2012-02-01

    We present a simple exactly solvable extension of the Jaynes-Cummings model by adding dissipation. This is done such that the total number of excitations is conserved. The Liouville operator in the resulting master equation can be reduced to blocks of 4×4 matrices.

  10. Excited states in hydrocarbons

    SciTech Connect

    Lipsky, S.

    1987-01-01

    In this brief review we first summarize some pertinent features of the photophysical properties of excited states of hydrocarbons and the mechanisms by which they transfer energy to solutes and then review their yields and their behavior under fast-electron irradiation conditions. 33 refs.

  11. Positron excitation of neon

    NASA Technical Reports Server (NTRS)

    Parcell, L. A.; Mceachran, R. P.; Stauffer, A. D.

    1990-01-01

    The differential and total cross section for the excitation of the 3s1P10 and 3p1P1 states of neon by positron impact were calculated using a distorted-wave approximation. The results agree well with experimental conclusions.

  12. Medium-frequency impulsive-thrust-excited slosh waves during propellant reorientation with a geyser

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.; Lee, C. C.

    1992-01-01

    Slosh wave excitation induced by a resettling flowfield activated by 1.0-Hz impulsive thrust during the course of liquid reorientation with the initiation of geyser for liquid-fill levels of 30, 50, 65, 70, and 80 percent has been studied. Characteristics of slosh waves of various frequencies excited by the resettling flowfield are discussed. Slosh wave excitations shift the fluid mass distribution in the container which imposes time-dependent variations in spacecraft moment of inertia. This information is important for spacecraft control during the course of liquid reorientation.

  13. A Novel Liquid-Liquid Transition in Undercooled Ti-Zr-Ni Liquids

    NASA Technical Reports Server (NTRS)

    Lee, G. W.; Gangopadhyay, A. K.; Kelton, K. F.; Bradshaw, R. C.; Hyers, R. W.; Rathz, T. J.; Rogers, J. R.

    2004-01-01

    If crystallization can be avoided, liquids enter a metastable (undercooled) state below their equilibrium liquidus temperatures, T(sub l), finally 'freezing' into a glass below a characteristic temperature called the glass transition temperature, T(sub g). In rare cases, the undercooled liquid may undergo a liquid-liquid phase transition (liquid polymorphism) before entering the glassy state. This has been suggested from experimental studies of H2O and Si. Such phase transitions have been predicted in some stable liquids, ie. above T(sub l) at atmospheric pressure, for SiO2 and BeF2, but these have not been verified experimentally. They have been observed in liquids of P, Si and C, but only under high pressure. In this letter we present the first experimental evidence for a phase transition in a low viscosity metallic liquid that is driven by an approach to a constant entropy configuration state and correlated with a growing icosahedral order in the liquid. A maximum in the specific heat at constant pressure, similar to what is normally observed near T(sub g), is reported for undercooled liquids of quasicrystal-forming Ti-Zr-Ni alloys. A two-state excitation model that includes cooperativity by incorporating a temperature-dependent excitation energy, fits the specific heat data well, signaling a phase transition. An inflection in the liquid density with decreasing temperature instead of a discontinuity indicates that this is not a typical first order phase transition; it could be a weakly first order or higher order transition. While showing many similarities to a glass transition, this liquid-liquid phase transition occurs in a mobile liquid, making it novel.

  14. Harmonically excited orbital variations

    SciTech Connect

    Morgan, T.

    1985-08-06

    Rephrasing the equations of motion for orbital maneuvers in terms of Lagrangian generalized coordinates instead of Newtonian rectangular cartesian coordinates can make certain harmonic terms in the orbital angular momentum vector more readily apparent. In this formulation the equations of motion adopt the form of a damped harmonic oscillator when torques are applied to the orbit in a variationally prescribed manner. The frequencies of the oscillator equation are in some ways unexpected but can nonetheless be exploited through resonant forcing functions to achieve large secular variations in the orbital elements. Two cases are discussed using a circular orbit as the control case: (1) large changes in orbital inclination achieved by harmonic excitation rather than one impulsive velocity change, and (2) periodic and secular changes to the longitude of the ascending node using both stable and unstable excitation strategies. The implications of these equations are also discussed for both artificial satellites and natural satellites. For the former, two utilitarian orbits are suggested, each exploiting a form of harmonic excitation. 5 refs.

  15. Aperture excited dielectric antennas

    NASA Technical Reports Server (NTRS)

    Crosswell, W. F.; Chatterjee, J. S.; Mason, V. B.; Tai, C. T.

    1974-01-01

    The results of a comprehensive experimental and theoretical study of the effect of placing dielectric objects over the aperture of waveguide antennas are presented. Experimental measurements of the radiation patterns, gain, impedance, near-field amplitude, and pattern and impedance coupling between pairs of antennas are given for various Plexiglas shapes, including the sphere and the cube, excited by rectangular, circular, and square waveguide feed apertures. The waveguide excitation of a dielectric sphere is modeled using the Huygens' source, and expressions for the resulting electric fields, directivity, and efficiency are derived. Calculations using this model show good overall agreement with experimental patterns and directivity measurements. The waveguide under an infinite dielectric slab is used as an impedance model. Calculations using this model agree qualitatively with the measured impedance data. It is concluded that dielectric loaded antennas such as the waveguide excited sphere, cube, or sphere-cylinder can produce directivities in excess of that obtained by a uniformly illuminated aperture of the same cross section, particularly for dielectric objects with dimensions of 2 wavelengths or less. It is also shown that for certain configurations coupling between two antennas of this type is less than that for the same antennas without dielectric loading.

  16. Internal waves excited by the marangoni effect

    PubMed

    Wierschem; Linde; Velarde

    2000-11-01

    Traveling periodic internal wave trains are generated in liquid layers during the absorption process of a miscible surface-active substance out of the vapor phase. In our nonstationary experimental runs, internal waves are excited by surface waves, which had been previously generated by a surface-tension-gradient-driven instability. The internal wave trains adjust their wave number by an Eckhaus instability. Close to the instability threshold narrow and extended pulses are observed. Furthermore, the wave trains can alter their traveling direction, i.e., one wave train traveling in one direction yields to another train, in general of different wave number, traveling in the opposite direction. PMID:11101989

  17. Photothermal excitation setup for a modified commercial atomic force microscope

    SciTech Connect

    Adam, Holger; Rode, Sebastian; Schreiber, Martin; Kühnle, Angelika; Kobayashi, Kei; Yamada, Hirofumi

    2014-02-15

    High-resolution imaging in liquids using frequency modulation atomic force microscopy is known to suffer from additional peaks in the resonance spectrum that are unrelated to the cantilever resonance. These unwanted peaks are caused by acoustic modes of the liquid and the setup arising from the indirect oscillation excitation by a piezoelectric transducer. Photothermal excitation has been identified as a suitable method for exciting the cantilever in a direct manner. Here, we present a simple design for implementing photothermal excitation in a modified Multimode scan head from Bruker. Our approach is based on adding a few components only to keep the modifications as simple as possible and to maintain the low noise level of the original setup with a typical deflection noise density of about 15 fm/√(Hz) measured in aqueous solution. The success of the modification is illustrated by a comparison of the resonance spectra obtained with piezoelectric and photothermal excitation. The performance of the systems is demonstrated by presenting high-resolution images on bare calcite in liquid as well as organic adsorbates (Alizarin Red S) on calcite with simultaneous atomic resolution of the underlying calcite substrate.

  18. SHOCK-EXCITED OSCILLATOR

    DOEpatents

    Creveling, R.

    1957-12-17

    S> A shock-excited quartz crystal oscillator is described. The circuit was specifically designed for application in micro-time measuring work to provide an oscillator which immediately goes into oscillation upon receipt of a trigger pulse and abruptly ceases oscillation when a second pulse is received. To achieve the instant action, the crystal has a prestressing voltage applied across it. A monostable multivibrator receives the on and off trigger pulses and discharges a pulse through the crystal to initiate or terminate oscillation instantly.

  19. Search for Gluonic Excitations

    SciTech Connect

    Paul Eugenio

    2007-10-01

    Studies of meson spectra via strong decays provide insight regarding QCD at the confinement scale. These studies have led to phenomenological models for QCD such as the constituent quark model. However, QCD allows for a much richer spectrum of meson states which include extra states such as exotics, hybrids, multi-quarks, and glueballs. First discussion of the status of exotic meson searches is given followed by a discussion of plans at Jefferson Lab to double the energy of the machine to 12 GeV, which will allow us to access photoproduction of mesons in search for gluonic excited states.

  20. Search for Gluonic Excitations

    SciTech Connect

    Eugenio, Paul

    2007-10-26

    Studies of meson spectra via strong decays provide insight regarding QCD at the confinement scale. These studies have led to phenomenological models for QCD such as the constituent quark model. However, QCD allows for a much richer spectrum of meson states which include extra states such as exotics, hybrids, multi-quarks, and glueballs. First discussion of the status of exotic meson searches is given followed by a discussion of plans at Jefferson Lab to double the energy of the machine to 12 GeV, which will allow us to access photoproduction of mesons in search for gluonic excited states.

  1. Nanotube Electron Drag in Flowing Liquids.

    PubMed

    Král; Shapiro

    2001-01-01

    We show that electric current can be generated in metallic carbon nanotubes immersed in liquids flowing along them. Molecular layers of the liquid coat the nanotube, slip along its surface, and excite there a phonon wind, which drags free carriers in the tube. The induced electric current should allow building of nanoscale detectors or power cells.

  2. Wigner Crystallization of Single Photons in Cold Rydberg Ensembles

    NASA Astrophysics Data System (ADS)

    Otterbach, Johannes; Moos, Matthias; Muth, Dominik; Fleischhauer, Michael

    2013-09-01

    The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency leads to the formation of Rydberg polaritons which are quasiparticles with tunable effective mass and nonlocal interactions. Confined to one spatial dimension their low energy physics is that of a moving-frame Luttinger liquid which, due to the nonlocal character of the repulsive interaction, can form a Wigner crystal of individual photons. We calculate the Luttinger K parameter using density-matrix renormalization group simulations and find that under typical slow-light conditions kinetic energy contributions are too strong for crystal formation. However, adiabatically increasing the polariton mass by turning a light pulse into stationary spin excitations allows us to generate true crystalline order over a finite length. The dynamics of this process and asymptotic correlations are analyzed in terms of a time-dependent Luttinger theory.

  3. Wigner crystallization of single photons in cold Rydberg ensembles.

    PubMed

    Otterbach, Johannes; Moos, Matthias; Muth, Dominik; Fleischhauer, Michael

    2013-09-13

    The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency leads to the formation of Rydberg polaritons which are quasiparticles with tunable effective mass and nonlocal interactions. Confined to one spatial dimension their low energy physics is that of a moving-frame Luttinger liquid which, due to the nonlocal character of the repulsive interaction, can form a Wigner crystal of individual photons. We calculate the Luttinger K parameter using density-matrix renormalization group simulations and find that under typical slow-light conditions kinetic energy contributions are too strong for crystal formation. However, adiabatically increasing the polariton mass by turning a light pulse into stationary spin excitations allows us to generate true crystalline order over a finite length. The dynamics of this process and asymptotic correlations are analyzed in terms of a time-dependent Luttinger theory. PMID:24074081

  4. Hydrological excitation of polar motion

    NASA Astrophysics Data System (ADS)

    Nastula, Y.; Kolaczek, B.

    2006-08-01

    Hydrological excitation of the polar motion (HAM) were computed from the available recently hydrological data series (NCEP, ECMWF, CPC water storage and LaD World simulations of global continental water) and compared. Time variable seasonal spectra of these hydrological excitation functions and of the geodetic excitation function of polar motion computed from the polar motion COMB03 data were compared showing big differences in their temporal characteristics and the necessity of the further improvement of the HAM models. Seasonal oscillations of the global geophysical excitation functions (AAM + OAM + HAM) and their time variations were compared also. These hydrological excitation functions do not close the budget of the global geophysical excitation function of polar motion.

  5. Neural Excitability and Singular Bifurcations.

    PubMed

    De Maesschalck, Peter; Wechselberger, Martin

    2015-12-01

    We discuss the notion of excitability in 2D slow/fast neural models from a geometric singular perturbation theory point of view. We focus on the inherent singular nature of slow/fast neural models and define excitability via singular bifurcations. In particular, we show that type I excitability is associated with a novel singular Bogdanov-Takens/SNIC bifurcation while type II excitability is associated with a singular Andronov-Hopf bifurcation. In both cases, canards play an important role in the understanding of the unfolding of these singular bifurcation structures. We also explain the transition between the two excitability types and highlight all bifurcations involved, thus providing a complete analysis of excitability based on geometric singular perturbation theory.

  6. Two-Gaussian excitations model for the glass transition

    NASA Astrophysics Data System (ADS)

    Matyushov, Dmitry V.; Angell, C. A.

    2005-07-01

    We develop a modified "two-state" model with Gaussian widths for the site energies of both ground and excited states, consistent with expectations for a disordered system. The thermodynamic properties of the system are analyzed in configuration space and found to bridge the gap between simple two-state models ("logarithmic" model in configuration space) and the random energy model ("Gaussian" model in configuration space). The Kauzmann singularity given by the random energy model remains for very fragile liquids but is suppressed or eliminated for stronger liquids. The sharp form of constant-volume heat capacity found by recent simulations for binary mixed Lennard-Jones and soft-sphere systems is reproduced by the model, as is the excess entropy and heat capacity of a variety of laboratory systems, strong and fragile. The ideal glass in all cases has a narrow Gaussian, almost invariant among molecular and atomic glassformers, while the excited-state Gaussian depends on the system and its width plays a role in the thermodynamic fragility. The model predicts the possibility of first-order phase transitions for fragile liquids. The analysis of laboratory data for toluene and o-terphenyl indicates that fragile liquids resolve the Kauzmann paradox by a first-order transition from supercooled liquid to ideal-glass state at a temperature between Tg and Kauzmann temperature extrapolated from experimental data. We stress the importance of the temperature dependence of the energy landscape, predicted by the fluctuation-dissipation theorem, in analyzing the liquid thermodynamics.

  7. Multiphonon excitations in boson quantum films

    SciTech Connect

    Clements, B.E. |; Krotscheck, E. |; Tymczak, C.J.

    1996-05-01

    Dynamical excitations in thin liquid films of {sup 4}He adsorbed to a substrate are investigated by using a microscopic theory of excitations that includes multiple-phonon scattering. We study the dispersion relation, excitation mechanisms, transition densities, and particle currents as a function of surface coverage. A primary new result is that we have included three-phonon scattering processes in the calculation of the dynamic structure function and the one-body current densities. With the exception that our ground state is determined by our variational theory, rather than taken from experiment, our work on the dynamic structure function is the generalization of that of Jackson [Phys. Rev. A {bold 4}, 2386 (1971)] to inhomogeneous systems (films). Using sum rules for the dynamic structure function as a guide, we suggest a simple scaling argument for improving the agreement between our dynamic structure function and the experimental one. The addition of three-phonon contributions bring about the following changes. First, the energy of most modes is lowered by a non-negligible amount for finite momentum excitations. Second, the film{close_quote}s surface mode is the exception; it is only slightly affected. Third, for monolayer films there is large scattering at high energies at intermediate values of momenta. This scattering can be traced back to an anomalously large contribution to the two-particle density of states. Fourth, all modes with energy above a critical energy decay, and the associated peaks of the dynamic structure function are broadened. Fifth, the maxonlike character is enhanced in the bulklike modes. {copyright} {ital 1996 The American Physical Society.}

  8. Electron excitations in solids and novel materials

    NASA Astrophysics Data System (ADS)

    Spataru, Catalin-Dan

    Several applications of the use of ab initio many-body methods in condensed matter theory are presented. In particular, these methods are used for the study of electronic excitations in various kinds of materials, ranging from bulk to low dimensional systems, and from metals to semiconductors. Two types of electron excitations are considered: quasiparticle excitations and electron-hole excitations. The work is organized in five chapters as follows: (1) The first chapter gives an introduction to the concept of quasiparticle and electron-hole excitations, as well as to the many-body framework underlying the theoretical formalism used in this work. (2) Chapter two presents the calculation of quasiparticle lifetimes in graphite. The inverse lifetime of low energy quasi-electrons shows significant deviations from the quadratic behavior naively expected from Fermi liquid theory. The deviations are explained in terms of the unique features of the band structure of this material. (3) In chapter three, the real and imaginary parts of the quasiparticle self-energy in jellium and crystalline Al are calculated at high electron temperatures. We find a decrease in the electron lifetime and an increase in the valence and conduction band widths as the temperature is increased. Calculation of the spectral function suggests that the quasiparticle concept may still be reasonable at high electron temperatures. (4) Chapter four presents calculations of the quasiparticle spectrum of highly irradiated crystalline GaAs. Our results indicate that the valence-conduction band gap is a sensitive function of the amount of electrons excited above the ground state. However, contrary to previous results, we find that it is not possible to induce a complete band gap closure by purely electronic means. (5) In chapter five we present calculations of the electron-hole interaction effects on the optical spectra of several single-walled carbon nanotubes. We show that the optical spectra of both

  9. Pattern Formation in Excitable Media

    NASA Astrophysics Data System (ADS)

    Reynolds, William Nash

    1992-01-01

    The phenomenon of excitability is observed in a wide variety of physical and biological systems. In this work, spatially extended excitable systems are examined from several different perspectives. First, a pedagogical introduction is used to motivate the derivation of the dynamics of one dimensional excitable pulses. In the second part, coupled map techniques for numerical simulation of excitable media and other interfacial systems are described. Examples are given for both excitable media and crystal growth. The third chapter addresses the phenomenon of spiral formation in excitable media. Exact rotating solutions are found for a class of models of excitable media. The solutions consist of two regions: an outer region, consisting of the spiral proper, which exhibits a singularity at its tip, and the core region, obtained by rescaling space in the vicinity of the tip. The tip singularity is resolved in the core region, leading to a consistent solution in all of space. The stability of both the spiral and the core is investigated, with the result that the spiral is found to be stable, and the core unstable. Finally, the stability of excitable waves of the chemical cAMP traveling over aggregating colonies of the slime mold Dictyostelium discoideum is examined by coupling the excitable dynamics of the cAMP signalling system to a simple model of chemotaxis, with result that cellular motion is found to destabilize the waves, causing the initially uniform field of cells to break up into streams.

  10. Fission fragment excited laser system

    DOEpatents

    McArthur, David A.; Tollefsrud, Philip B.

    1976-01-01

    A laser system and method for exciting lasing action in a molecular gas lasing medium which includes cooling the lasing medium to a temperature below about 150 K and injecting fission fragments through the lasing medium so as to preferentially excite low lying vibrational levels of the medium and to cause population inversions therein. The cooled gas lasing medium should have a mass areal density of about 5 .times. 10.sup.-.sup.3 grams/square centimeter, relaxation times of greater than 50 microseconds, and a broad range of excitable vibrational levels which are excitable by molecular collisions.

  11. Excited State Dynamics of 7-AZAINDOLE Homodimer in Frozen Nitrogen Matrix

    NASA Astrophysics Data System (ADS)

    Mukherjee, Moitrayee; Bandyopadhyay, Biman; Karmakar, Shreetama; Chakraborty, Tapas

    2011-06-01

    In a fluid medium (liquid or gas), the doubly hydrogen bonded dimer of 7-azaindole (7AI) undergoes tautomerization via simultaneous exchange of two H-atoms/protons between the two moieties upon UV excitation to lowest excited singlet state. The excited dimer emits exclusively visible fluorescence from tautomeric configuration, and no UV fluorescence is detected from the locally excited state. We show here for the first time that this generic excited state dynamics of 7AI dimer is totally altered if the species is synthesized and confined in frozen nitrogen at 8 K. The dimer has been found to emit only from the locally excited state, and the photophysical channel leading to excited state tautomerization is completely blocked. The formation of the centrosymmetric dimer in nitrogen matrix is ensured by recording the FTIR spectrum of the dimer before initiating the photophysical measurements. The details of our findings and interpretation of the measured data will be presented in the talk.

  12. Collective excitations in soft-sphere fluids.

    PubMed

    Bryk, Taras; Gorelli, Federico; Ruocco, Giancarlo; Santoro, Mario; Scopigno, Tullio

    2014-10-01

    Despite that the thermodynamic distinction between a liquid and the corresponding gas ceases to exist at the critical point, it has been recently shown that reminiscence of gaslike and liquidlike behavior can be identified in the supercritical fluid region, encoded in the behavior of hypersonic waves dispersion. By using a combination of molecular dynamics simulations and calculations within the approach of generalized collective modes, we provide an accurate determination of the dispersion of longitudinal and transverse collective excitations in soft-sphere fluids. Specifically, we address the decreasing rigidity upon density reduction along an isothermal line, showing that the positive sound dispersion, an excess of sound velocity over the hydrodynamic limit typical for dense liquids, displays a nonmonotonic density dependence strictly correlated to that of thermal diffusivity and kinematic viscosity. This allows rationalizing recent observation parting the supercritical state based on the Widom line, i.e., the extension of the coexistence line. Remarkably, we show here that the extremals of transport properties such as thermal diffusivity and kinematic viscosity provide a robust definition for the boundary between liquidlike and gaslike regions, even in those systems without a liquid-gas binodal line. Finally, we discuss these findings in comparison with recent results for Lennard-Jones model fluid and with the notion of the "rigid-nonrigid" fluid separation lines.

  13. Probing liquid surface waves, liquid properties and liquid films with light diffraction

    NASA Astrophysics Data System (ADS)

    Barik, Tarun Kr; Chaudhuri, Partha Roy; Roy, Anushree; Kar, Sayan

    2006-06-01

    Surface waves on liquids act as a dynamical phase grating for incident light. In this paper, we revisit the classical method of probing such waves (wavelengths of the order of mm) as well as inherent properties of liquids and liquid films on liquids, using optical diffraction. A combination of simulation and experiment is proposed to trace out the surface wave profiles in various situations (e.g. for one or more vertical, slightly immersed, electrically driven exciters). Subsequently, the surface tension and the spatial damping coefficient (related to viscosity) of a variety of liquids are measured carefully in order to gauge the efficiency of measuring liquid properties using this optical probe. The final set of results deal with liquid films where dispersion relations, surface and interface modes, interfacial tension and related issues are investigated in some detail, both theoretically and experimentally. On the whole, our observations and analysis seem to support the claim that this simple, low cost apparatus is capable of providing a wealth of information on liquids and liquid surface waves in a non-destructive way.

  14. A Liquid-Liquid Transition in an Undercooled Ti-Zr-Ni Liquid

    NASA Technical Reports Server (NTRS)

    Lee, G. W.; Gangopadhyay, A. K.; Kelton, K. F.; Hyers, R. W.; Rathz, T. J.; Rogers, J. R.

    2003-01-01

    If crystallization can be avoided, liquids enter a metastable (undercooled) state below their equilibrium liquidus temperatures, TI, finally freezing into a glass below a characteristic temperature called the glass transition temperature, T,. In rare cases, the undercooled liquid may undergo a liquid-liquid phase transition (liquid polymorphism) before entering the glassy state. This has been suggested from experimental studies of HzO and Si4. Such phase transitions have been predicted in some stable liquids, i.e. above TI at atmospheric pressure, for Si02 and BeF;, but these have not been verified experimentally. They have been observed in liquids of P7, Sis and C9, but only under high pressure. All of these transitions are driven by an anomalous density change, i.e. change in local structure, with temperature or pressure. In this letter we present the first experimental evidence for a phase transition in a low viscosity liquid that is not driven by an anomalous density change, but by an approach to a constant configuration state. A maximum in the specific heat at constant pressure, similar to what is normally observed near T,, is reported here for undercooled low viscosity liquids of quasicrystal- forming Ti-Zr-Ni alloys. that includes cooperativity, by incorporating a temperature dependent excitation energy fits the data well, signaling a phase transition.

  15. Coulomb excitation of 31Mg

    NASA Astrophysics Data System (ADS)

    Seidlitz, M.; Mücher, D.; Reiter, P.; Bildstein, V.; Blazhev, A.; Bree, N.; Bruyneel, B.; Cederkäll, J.; Clement, E.; Davinson, T.; Van Duppen, P.; Ekström, A.; Finke, F.; Fraile, L. M.; Geibel, K.; Gernhäuser, R.; Hess, H.; Holler, A.; Huyse, M.; Ivanov, O.; Jolie, J.; Kalkühler, M.; Kotthaus, T.; Krücken, R.; Lutter, R.; Piselli, E.; Scheit, H.; Stefanescu, I.; Van de Walle, J.; Voulot, D.; Warr, N.; Wenander, F.; Wiens, A.

    2011-06-01

    The ground state properties of 31Mg indicate a change of nuclear shape at N = 19 with a deformed Jπ = 1 /2+ intruder state as a ground state, implying that 31Mg is part of the "island of inversion". The collective properties of excited states were the subject of a Coulomb excitation experiment at REX-ISOLDE, CERN, employing a radioactive 31Mg beam. De-excitation γ-rays were detected by the MINIBALL γ-spectrometer in coincidence with scattered particles in a segmented Si-detector. The level scheme of 31Mg was extended. Spin and parity assignment of the 945 keV state yielded 5 /2+ and its de-excitation is dominated by a strong collective M1 transition. Comparison of the transition probabilities of 30,31,32Mg establishes that for the N = 19 magnesium isotope not only the ground state but also excited states are largely dominated by a deformed pf intruder configuration.

  16. Excited waves in shear layers

    NASA Technical Reports Server (NTRS)

    Bechert, D. W.

    1982-01-01

    The generation of instability waves in free shear layers is investigated. The model assumes an infinitesimally thin shear layer shed from a semi-infinite plate which is exposed to sound excitation. The acoustical shear layer excitation by a source further away from the plate edge in the downstream direction is very weak while upstream from the plate edge the excitation is relatively efficient. A special solution is given for the source at the plate edge. The theory is then extended to two streams on both sides of the shear layer having different velocities and densities. Furthermore, the excitation of a shear layer in a channel is calculated. A reference quantity is found for the magnitude of the excited instability waves. For a comparison with measurements, numerical computations of the velocity field outside the shear layer were carried out.

  17. Vibrational excitation induces double reaction.

    PubMed

    Huang, Kai; Leung, Lydie; Lim, Tingbin; Ning, Zhanyu; Polanyi, John C

    2014-12-23

    Electron-induced reaction at metal surfaces is currently the subject of extensive study. Here, we broaden the range of experimentation to a comparison of vibrational excitation with electronic excitation, for reaction of the same molecule at the same clean metal surface. In a previous study of electron-induced reaction by scanning tunneling microscopy (STM), we examined the dynamics of the concurrent breaking of the two C-I bonds of ortho-diiodobenzene physisorbed on Cu(110). The energy of the incident electron was near the electronic excitation threshold of E0=1.0 eV required to induce this single-electron process. STM has been employed in the present work to study the reaction dynamics at the substantially lower incident electron energies of 0.3 eV, well below the electronic excitation threshold. The observed increase in reaction rate with current was found to be fourth-order, indicative of multistep reagent vibrational excitation, in contrast to the first-order rate dependence found earlier for electronic excitation. The change in mode of excitation was accompanied by altered reaction dynamics, evidenced by a different pattern of binding of the chemisorbed products to the copper surface. We have modeled these altered reaction dynamics by exciting normal modes of vibration that distort the C-I bonds of the physisorbed reagent. Using the same ab initio ground potential-energy surface as in the prior work on electronic excitation, but with only vibrational excitation of the physisorbed reagent in the asymmetric stretch mode of C-I bonds, we obtained the observed alteration in reaction dynamics.

  18. Two-photon excitation in laser scanning fluorescence microscopy

    NASA Astrophysics Data System (ADS)

    Strickler, James H.; Webb, Watt W.

    1991-04-01

    Simultaneous absorption of two red photons from a strongly focused subpicosecond colliding pulse mode4ocked dye laser stimulates visible fluorescence emission from fluorophores having their normal absorption in the ultraviolet1. The quadratic increase of the two-photon excitation rate with excitation intensity restricts fluorescence emission to the focal volume thus providing the same depth resolution as does confocal microscopy. Image degradation due to out of focus backround is thus avoided. Photobleaching and most cellular photodamage are similarly confined to the focus thereby minimizing sample degredation during acquisition of the multiple sections required for 3-d image reconstruction. Fluorescence images of living cells and other thick photolabile fluorescence labled assemblies illustrate the depth discrimination of both two-photon fluorescence excitation and photobleaching. The quadratic intensity dependence of two-photon excitation allows 3-d spatially resolved photochemistry in particular the photolytic release of caged compounds such as neurotransmitters nucleotides fluorescent dyes and second messengers such as 1P3 and Ca. The two-photon release of cased ATP has been measured and release of a caged fluorescent dye has been shown. Point photobleaching and a 3-d " write once read many" optical memory have been demonstrated. Two-photon excitation of photo-initiated polymerization with a sharply focused single beam allows microfabrication of complex structures of arbitrary form. By scanning the focused beam through a liquid polymer with a UV excited initiator it is possible to harden the polymer only at the focus thereby creating

  19. Coalescence of Liquid Drops

    NASA Technical Reports Server (NTRS)

    Yao, Wei-Jun

    2003-01-01

    When two liquid drops come into contact, a neck forms between them and grows rapidly. We are interested in the very early stage of the coalescence process, which can be characterized by the time dependence of the radius of the neck. The functional dependence of the size of the neck on time depends on the properties of the liquid. Experimentally, we are investigating a liquid in Stokes flow regime where the viscosity provides the principal retarding force to the surface tension. Recently, it has been predicted that the neck radius should change as t ln|t| in this regime. Theoretically, we have studied the situation when the velocity at each point on the surface is proportional to the local curvature and directed normal to the surface. This is the case that should be applicable to superfluid helium at low temperature when the mean free path of the thermal excitations are comparable to the size of liquid drops. For this system, the radius of the neck is found to be proportional to t(sup 1/3). We are able to find a simple expression for the shape of the interface in the vicinity of the neck.

  20. Fluorescent optical liquid level sensor

    DOEpatents

    Weiss, Jonathan D.

    2001-01-01

    A liquid level sensor comprising a transparent waveguide containing fluorescent material that is excited by light of a first wavelength and emits at a second, longer wavelength. The upper end of the waveguide is connected to a light source at the first wavelength through a beveled portion of the waveguide such that the input light is totally internally reflected within the waveguide above an air/liquid interface in a tank but is transmitted into the liquid below this interface. Light is emitted from the fluorescent material only in those portions of the waveguide that are above the air/liquid interface, to be collected at the upper end of the waveguide by a detector that is sensitive only to the second wavelength. As the interface moves down in the tank, the signal strength from the detector will increase.

  1. Coulomb excitation of 107In

    NASA Astrophysics Data System (ADS)

    DiJulio, D. D.; Cederkall, J.; Fahlander, C.; Ekström, A.; Hjorth-Jensen, M.; Albers, M.; Bildstein, V.; Blazhev, A.; Darby, I.; Davinson, T.; De Witte, H.; Diriken, J.; Fransen, Ch.; Geibel, K.; Gernhäuser, R.; Görgen, A.; Hess, H.; Heyde, K.; Iwanicki, J.; Lutter, R.; Reiter, P.; Scheck, M.; Seidlitz, M.; Siem, S.; Taprogge, J.; Tveten, G. M.; Van de Walle, J.; Voulot, D.; Warr, N.; Wenander, F.; Wimmer, K.

    2013-01-01

    The radioactive isotope 107In was studied using sub-barrier Coulomb excitation at the REX-ISOLDE facility at CERN. Two γ rays were observed during the experiment, corresponding to the low-lying 11/2+ and 3/2- states. The reduced transition probability of the 11/2+ state was determined with the semiclassical Coulomb excitation code gosia2. The result is discussed in comparison to large-scale shell-model calculations, previous unified-model calculations, and earlier Coulomb excitation measurements in the odd-mass In isotopes.

  2. LIQUID-LIQUID EXTRACTION COLUMNS

    DOEpatents

    Thornton, J.D.

    1957-12-31

    This patent relates to liquid-liquid extraction columns having a means for pulsing the liquid in the column to give it an oscillatory up and down movement, and consists of a packed column, an inlet pipe for the dispersed liquid phase and an outlet pipe for the continuous liquid phase located in the direct communication with the liquid in the lower part of said column, an inlet pipe for the continuous liquid phase and an outlet pipe for the dispersed liquid phase located in direct communication with the liquid in the upper part of said column, a tube having one end communicating with liquid in the lower part of said column and having its upper end located above the level of said outlet pipe for the dispersed phase, and a piston and cylinder connected to the upper end of said tube for applying a pulsating pneumatic pressure to the surface of the liquid in said tube so that said surface rises and falls in said tube.

  3. Solvation of electronically excited I2 -

    NASA Astrophysics Data System (ADS)

    Maslen, P. E.; Papanikolas, J. M.; Faeder, J.; Parson, R.; ONeil, S. V.

    1994-10-01

    The interaction potentials between the six lowest electronic states of I-2 and an arbitrary discrete charge distribution are calculated approximately using a one-electron model. The model potentials are much easier to calculate than ab initio potentials, with the cost of a single energy point scaling linearly with the number of solvent molecules, enabling relatively large systems to be studied. Application of the model to simulation of electronically excited I-2 in liquids and CO2 clusters is discussed. In a preliminary application, solvent effects are approximated by a uniform electric field. If electronically excited (2Πg,1/2) I-2 undergoes dissociation in the presence of a strong electric field, the negative charge localizes so as to minimize the total potential energy. However, in a weak field the negative charge localizes in the opposite direction, maximizing the potential energy. Based on a study of the field-dependent potential surfaces, a solvent-transfer mechanism is proposed for the electronic relaxation of 2Πg,1/2I-2, in contrast to the conventional view of relaxation via electron transfer.

  4. LSPR properties of metal nanoparticles adsorbed at a liquid-liquid interface.

    PubMed

    Yang, Zhilin; Chen, Shu; Fang, Pingping; Ren, Bin; Girault, Hubert H; Tian, Zhongqun

    2013-04-21

    Unlike the solid-air and solid-liquid interfaces, the optical properties of metal nanoparticles adsorbed at the liquid-liquid interface have not been theoretically exploited to date. In this work, the three dimensional finite difference time domain (3D-FDTD) method is employed to clarify the localized surface plasmon resonance (LSPR) based optical properties of gold nanoparticles (NPs) adsorbed at the water-oil interface, including near field distribution, far field absorption and their relevance. The LSPR spectra of NPs located at a liquid-liquid interface are shown to differ significantly from those in a uniform liquid environment or at the other interfaces. The absorption spectra exhibit two distinct LSPR peaks, the positions and relative strengths of which are sensitive to the dielectric properties of each liquid and the exact positions of the NPs with respect to the interface. Precise control of the particles' position and selection of the appropriate wavelength of the excitation laser facilitates the rational design and selective excitation of localized plasmon modes for interfacial NPs, a necessary advance for the exploration of liquid-liquid interfaces via surface enhanced Raman spectroscopy (SERS). According to our calculations, the SERS enhancement factor for Au nanosphere dimers at the water-oil interface can be as high as 10(7)-10(9), implying significant promise for future investigations of interfacial structure and applications of liquid-liquid interfaces towards chemical analysis.

  5. Resonance Radiation and Excited Atoms

    NASA Astrophysics Data System (ADS)

    Mitchell, Allan C. G.; Zemansky, Mark W.

    2009-06-01

    1. Introduction; 2. Physical and chemical effects connected with resonance radiation; 3. Absorption lines and measurements of the lifetime of the resonance state; 4. Collision processes involving excited atoms; 5. The polarization of resonance radiation; Appendix; Index.

  6. Collisional excitation of interstellar formaldehyde

    NASA Technical Reports Server (NTRS)

    Green, S.; Garrison, B. J.; Lester, W. A., Jr.; Miller, W. H.

    1978-01-01

    Previous calculations for rates of excitation of ortho-H2CO by collisions with He have been extended to higher rotational levels and kinetic temperatures to 80 K. Rates for para-H2CO have also been computed. Pressure-broadening widths for several spectral lines have been obtained from these calculations and are found to agree with recent data within the experimental uncertainty of 10%. Excitation of formaldehyde by collisions with H2 molecules is also discussed.

  7. Excitations of strange bottom baryons

    NASA Astrophysics Data System (ADS)

    Woloshyn, R. M.

    2016-09-01

    The ground-state and first-excited-state masses of Ωb and Ω_{bb} baryons are calculated in lattice QCD using dynamical 2 + 1 flavour gauge fields. A set of baryon operators employing different combinations of smeared quark fields was used in the framework of the variational method. Results for radial excitation energies were confirmed by carrying out a supplementary multiexponential fitting analysis. Comparison is made with quark model calculations.

  8. Exciting Polaritons with Quantum Light.

    PubMed

    López Carreño, J C; Sánchez Muñoz, C; Sanvitto, D; del Valle, E; Laussy, F P

    2015-11-01

    We discuss the excitation of polaritons-strongly coupled states of light and matter-by quantum light, instead of the usual laser or thermal excitation. As one illustration of the new horizons thus opened, we introduce "Mollow spectroscopy"-a theoretical concept for a spectroscopic technique that consists of scanning the output of resonance fluorescence onto an optical target-from which weak nonlinearities can be read with high precision even in strongly dissipative environments. PMID:26588401

  9. Electron-excited molecule interactions

    SciTech Connect

    Christophorou, L.G. Tennessee Univ., Knoxville, TN . Dept. of Physics)

    1991-01-01

    In this paper the limited but significant knowledge to date on electron scattering from vibrationally/rotationally excited molecules and electron scattering from and electron impact ionization of electronically excited molecules is briefly summarized and discussed. The profound effects of the internal energy content of a molecule on its electron attachment properties are highlighted focusing in particular on electron attachment to vibrationally/rotationally and to electronically excited molecules. The limited knowledge to date on electron-excited molecule interactions clearly shows that the cross sections for certain electron-molecule collision processes can be very different from those involving ground state molecules. For example, optically enhanced electron attachment studies have shown that electron attachment to electronically excited molecules can occur with cross sections 10{sup 6} to 10{sup 7} times larger compared to ground state molecules. The study of electron-excited molecule interactions offers many experimental and theoretical challenges and opportunities and is both of fundamental and technological significance. 54 refs., 15 figs.

  10. Redox Control of Cardiac Excitability

    PubMed Central

    Aggarwal, Nitin T.

    2013-01-01

    Abstract Reactive oxygen species (ROS) have been associated with various human diseases, and considerable attention has been paid to investigate their physiological effects. Various ROS are synthesized in the mitochondria and accumulate in the cytoplasm if the cellular antioxidant defense mechanism fails. The critical balance of this ROS synthesis and antioxidant defense systems is termed the redox system of the cell. Various cardiovascular diseases have also been affected by redox to different degrees. ROS have been indicated as both detrimental and protective, via different cellular pathways, for cardiac myocyte functions, electrophysiology, and pharmacology. Mostly, the ROS functions depend on the type and amount of ROS synthesized. While the literature clearly indicates ROS effects on cardiac contractility, their effects on cardiac excitability are relatively under appreciated. Cardiac excitability depends on the functions of various cardiac sarcolemal or mitochondrial ion channels carrying various depolarizing or repolarizing currents that also maintain cellular ionic homeostasis. ROS alter the functions of these ion channels to various degrees to determine excitability by affecting the cellular resting potential and the morphology of the cardiac action potential. Thus, redox balance regulates cardiac excitability, and under pathological regulation, may alter action potential propagation to cause arrhythmia. Understanding how redox affects cellular excitability may lead to potential prophylaxis or treatment for various arrhythmias. This review will focus on the studies of redox and cardiac excitation. Antioxid. Redox Signal. 18, 432–468. PMID:22897788

  11. Coherent control of multiple vibrational excitations for optimal detection

    NASA Astrophysics Data System (ADS)

    McGrane, S. D.; Scharff, R. J.; Greenfield, M.; Moore, D. S.

    2009-10-01

    While the means to selectively excite a single vibrational mode using ultrafast pulse shaping are well established, the subsequent problem of selectively exciting multiple vibrational modes simultaneously has been largely neglected. The coherent control of multiple vibrational excitations has applications in control of chemistry, chemical detection and molecular vibrational quantum information processing. Using simulations and experiments, we demonstrate that multiple vibrational modes can be selectively excited with the concurrent suppression of multiple interfering modes by orders of magnitude. While the mechanism of selectivity is analogous to that of single mode selectivity, the interferences required to select multiple modes require complicated non-intuitive pulse trains. Additionally, we show that selective detection can be achieved by the optimal pulse shape, even when the nature of the interfering species is varied, suggesting that optimized detection should be practical in real world applications. Experimental measurements of the multiplex coherent anti-Stokes Raman spectra (CARS) and CARS decay times of toluene, acetone, cis-stilbene and nitromethane liquids are reported, along with optimizations attempting to selectively excite nitromethane in a mixture of the four solvents. The experimental implementation exhibits a smaller degree of signal to background enhancement than predicted, which is primarily attributed to the single objective optimization methodology and not to fundamental limitations.

  12. Liquid metal thermoacoustic engine

    SciTech Connect

    Swift, G.W.; Migliori, A.; Wheatley, J.C.

    1986-01-01

    We are studying a liquid metal thermoacoustic engine both theoretically and experimentally. This type of engine promises to produce large quantities of electrical energy from heat at modest efficiency with no moving parts. A sound wave is usually thought of as consisting of pressure oscillations, but always attendant to the pressure oscillation are temperature oscillations. The combination produces a rich variety of ''thermoacoustic'' effects. These effects are usually so small that they are never noticed in everyday life; nevertheless under the right circumstances they can be harnessed to produce powerful heat engines, heat pumps, and refrigerators. In our liquid metal thermoacoustic engine, heat flow from a high temperature source to a low temperature sink generates a high-amplitude standing acoustic wave in liquid sodium. This acoustic power is converted to electric power by a simple magnetohydrodynamic effect at the acoustic oscillation frequency. We have developed a detailed thermoacoustic theory applicable to this engine, and find that a reasonably designed liquid sodium engine operating between 700/sup 0/C and 100/sup 0/C should generate about 60 W/cm/sup 2/ of acoustic power at about 1/3 of Carnot's efficiency. Construction of a 3000 W-thermal laboratory model engine has just been completed, and we have exciting preliminary experimental results as of the time of preparation of this manuscript showing, basically, that the engine works. We have also designed and built a 1 kHz liquid sodium magnetohydrodynamic generator and have extensive measurements on it. It is now very well characterized both experimentally and theoretically. The first generator of its kind, it already converts acoustic power to electric power with 40% efficiency. 16 refs., 5 figs.

  13. Liquid Ventilation

    PubMed Central

    Tawfic, Qutaiba A.; Kausalya, Rajini

    2011-01-01

    Mammals have lungs to breathe air and they have no gills to breath liquids. When the surface tension at the air-liquid interface of the lung increases, as in acute lung injury, scientists started to think about filling the lung with fluid instead of air to reduce the surface tension and facilitate ventilation. Liquid ventilation (LV) is a technique of mechanical ventilation in which the lungs are insufflated with an oxygenated perfluorochemical liquid rather than an oxygen-containing gas mixture. The use of perfluorochemicals, rather than nitrogen, as the inert carrier of oxygen and carbon dioxide offers a number of theoretical advantages for the treatment of acute lung injury. In addition, there are non-respiratory applications with expanding potential including pulmonary drug delivery and radiographic imaging. The potential for multiple clinical applications for liquid-assisted ventilation will be clarified and optimized in future. PMID:22043370

  14. LIQUID TARGET

    DOEpatents

    Martin, M.D.; Salsig, W.W. Jr.

    1959-01-13

    A liquid handling apparatus is presented for a liquid material which is to be irradiated. The apparatus consists essentially of a reservoir for the liquid, a target element, a drain tank and a drain lock chamber. The target is in the form of a looped tube, the upper end of which is adapted to be disposed in a beam of atomic particles. The lower end of the target tube is in communication with the liquid in the reservoir and a means is provided to continuously circulate the liquid material to be irradiated through the target tube. Means to heat the reservoir tank is provided in the event that a metal is to be used as the target material. The apparatus is provided with suitable valves and shielding to provide maximum safety in operation.

  15. Indirect excitation of ultrafast demagnetization

    PubMed Central

    Vodungbo, Boris; Tudu, Bahrati; Perron, Jonathan; Delaunay, Renaud; Müller, Leonard; Berntsen, Magnus H.; Grübel, Gerhard; Malinowski, Grégory; Weier, Christian; Gautier, Julien; Lambert, Guillaume; Zeitoun, Philippe; Gutt, Christian; Jal, Emmanuelle; Reid, Alexander H.; Granitzka, Patrick W.; Jaouen, Nicolas; Dakovski, Georgi L.; Moeller, Stefan; Minitti, Michael P.; Mitra, Ankush; Carron, Sebastian; Pfau, Bastian; von Korff Schmising, Clemens; Schneider, Michael; Eisebitt, Stefan; Lüning, Jan

    2016-01-01

    Does the excitation of ultrafast magnetization require direct interaction between the photons of the optical pump pulse and the magnetic layer? Here, we demonstrate unambiguously that this is not the case. For this we have studied the magnetization dynamics of a ferromagnetic cobalt/palladium multilayer capped by an IR-opaque aluminum layer. Upon excitation with an intense femtosecond-short IR laser pulse, the film exhibits the classical ultrafast demagnetization phenomenon although only a negligible number of IR photons penetrate the aluminum layer. In comparison with an uncapped cobalt/palladium reference film, the initial demagnetization of the capped film occurs with a delayed onset and at a slower rate. Both observations are qualitatively in line with energy transport from the aluminum layer into the underlying magnetic film by the excited, hot electrons of the aluminum film. Our data thus confirm recent theoretical predictions. PMID:26733106

  16. Indirect excitation of ultrafast demagnetization.

    PubMed

    Vodungbo, Boris; Tudu, Bharati; Tudu, Bahrati; Perron, Jonathan; Delaunay, Renaud; Müller, Leonard; Berntsen, Magnus H; Grübel, Gerhard; Malinowski, Grégory; Weier, Christian; Gautier, Julien; Lambert, Guillaume; Zeitoun, Philippe; Gutt, Christian; Jal, Emmanuelle; Reid, Alexander H; Granitzka, Patrick W; Jaouen, Nicolas; Dakovski, Georgi L; Moeller, Stefan; Minitti, Michael P; Mitra, Ankush; Carron, Sebastian; Pfau, Bastian; von Korff Schmising, Clemens; Schneider, Michael; Eisebitt, Stefan; Lüning, Jan

    2016-01-01

    Does the excitation of ultrafast magnetization require direct interaction between the photons of the optical pump pulse and the magnetic layer? Here, we demonstrate unambiguously that this is not the case. For this we have studied the magnetization dynamics of a ferromagnetic cobalt/palladium multilayer capped by an IR-opaque aluminum layer. Upon excitation with an intense femtosecond-short IR laser pulse, the film exhibits the classical ultrafast demagnetization phenomenon although only a negligible number of IR photons penetrate the aluminum layer. In comparison with an uncapped cobalt/palladium reference film, the initial demagnetization of the capped film occurs with a delayed onset and at a slower rate. Both observations are qualitatively in line with energy transport from the aluminum layer into the underlying magnetic film by the excited, hot electrons of the aluminum film. Our data thus confirm recent theoretical predictions. PMID:26733106

  17. Indirect excitation of ultrafast demagnetization

    DOE PAGES

    Vodungbo, Boris; Tudu, Bahrati; Perron, Jonathan; Delaunay, Renaud; Müller, Leonard; Berntsen, Magnus H.; Grübel, Gerhard; Malinowski, Grégory; Weier, Christian; Gautier, Julien; et al

    2016-01-06

    Does the excitation of ultrafast magnetization require direct interaction between the photons of the optical pump pulse and the magnetic layer? Here, we demonstrate unambiguously that this is not the case. For this we have studied the magnetization dynamics of a ferromagnetic cobalt/palladium multilayer capped by an IR-opaque aluminum layer. Upon excitation with an intense femtosecond-short IR laser pulse, the film exhibits the classical ultrafast demagnetization phenomenon although only a negligible number of IR photons penetrate the aluminum layer. In comparison with an uncapped cobalt/palladium reference film, the initial demagnetization of the capped film occurs with a delayed onset andmore » at a slower rate. Both observations are qualitatively in line with energy transport from the aluminum layer into the underlying magnetic film by the excited, hot electrons of the aluminum film. As a result, our data thus confirm recent theoretical predictions.« less

  18. Recurrent Excitation in Neocortical Circuits

    NASA Astrophysics Data System (ADS)

    Douglas, Rodney J.; Koch, Christof; Mahowald, Misha; Martin, Kevan A. C.; Suarez, Humbert H.

    1995-08-01

    The majority of synapses in the mammalian cortex originate from cortical neurons. Indeed, the largest input to cortical cells comes from neighboring excitatory cells. However, most models of cortical development and processing do not reflect the anatomy and physiology of feedback excitation and are restricted to serial feedforward excitation. This report describes how populations of neurons in cat visual cortex can use excitatory feedback, characterized as an effective "network conductance," to amplify their feedforward input signals and demonstrates how neuronal discharge can be kept proportional to stimulus strength despite strong, recurrent connections that threaten to cause runaway excitation. These principles are incorporated into models of cortical direction and orientation selectivity that emphasize the basic design principles of cortical architectures.

  19. Excitation optimization for damage detection

    SciTech Connect

    Bement, Matthew T; Bewley, Thomas R

    2009-01-01

    A technique is developed to answer the important question: 'Given limited system response measurements and ever-present physical limits on the level of excitation, what excitation should be provided to a system to make damage most detectable?' Specifically, a method is presented for optimizing excitations that maximize the sensitivity of output measurements to perturbations in damage-related parameters estimated with an extended Kalman filter. This optimization is carried out in a computationally efficient manner using adjoint-based optimization and causes the innovations term in the extended Kalman filter to be larger in the presence of estimation errors, which leads to a better estimate of the damage-related parameters in question. The technique is demonstrated numerically on a nonlinear 2 DOF system, where a significant improvement in the damage-related parameter estimation is observed.

  20. Pair Excitations in Fermi Fluids

    NASA Astrophysics Data System (ADS)

    Böhm, Helga M.; Krotscheck, Eckhard; Schörkhuber, Karl; Springer, Josef

    2006-09-01

    We present a theory of multi-pair excitations in strongly interacting Fermi systems. Based on an equations-of-motion approach for time-dependent pair correlations it leads to a qualitatively new structure of the density-density response function. Our theory reduces to both, i) the "correlated" random-phase approximation (RPA) for fermions if the two-pair excitations are ignored, and ii) the correlated Brillouin-Wigner perturbation theory for bosons in the appropriate limit. The theory preserves the two first energy-weighted sum rules. A familiar problem of the standard RPA is that its zero-sound mode is energetically much higher than found in experiments. The popular cure of introducing an average effective mass in the Lindhard function violates sum rules and describes the physics incorrectly. We demonstrate that the inclusion of correlated pair excitations gives the correct dispersion. As in 4He, a modification of the effective mass is unnecessary also in 3He.

  1. Calculation of molecular excitation rates

    NASA Astrophysics Data System (ADS)

    Flynn, George

    1993-01-01

    State-to-state collisional excitation rates for interstellar molecules observed by radio astronomers continue to be required to interpret observed line intensities in terms of local temperatures and densities. A problem of particular interest is collisional excitation of water which is important for modeling the observed interstellar masers. In earlier work supported by a different NASA Grant, excitation of water in collisions with He atoms was studied; after many years of successively more refined calculations that problem now seems to be well understood, and discrepancies with earlier experimental data for related (pressure broadening) phenomena are believed to reflect experimental errors. Because of interstellar abundances, excitation by H2, the dominant interstellar species, is much more important than excitation by He, although it has been argued that rates for excitation by these are similar. Under the current grant theoretical study of this problem has begun which is greatly complicated by the additional degrees of freedom which must be included both in determining the interaction potential and also in the molecular scattering calculation. We have now computed the interaction forces for nearly a thousand molecular geometries and are close to having an acceptable global fit to these points which is necessary for the molecular dynamics calculations. Also, extensive modifications have been made to the molecular scattering code, MOLSCAT. These included coding the rotational basis sets and coupling matrix elements required for collisions of an asymmetric top with a linear rotor. A new method for numerical solution of the coupled equations has been incorporated. Because of the long-ranged nature of the water-hydrogen interaction it is necessary to integrate the equations to rather large intermolecular separations, and the integration methods previously available in MOLSCAT are not ideal for such cases. However, the method used by Alexander in his HIBRIDON code is

  2. Magnetically induced pulser laser excitation

    SciTech Connect

    Taylor, R.S.; Leopold, K.E.

    1985-02-15

    A novel excitation scheme has been developed for excimer discharge lasers. The technique uses pulse transformer technology to induce a fast, high voltage pulse directly onto a ground potential laser electrode resulting in the breakdown of the laser gas mix. Saturation of the pulse transformer core inductance then permits efficient energy transfer from the main energy storage circuit into the discharge. When this excitation technique was used in a XeCl laser an output energy density of 2.5 J/l and an overall electrical to optical efficiency of 2% were obtained. The technique appears promising for the development of high energy, high average power excimer lasers.

  3. Autoresonant excitation of antiproton plasmas.

    PubMed

    Andresen, G B; Ashkezari, M D; Baquero-Ruiz, M; Bertsche, W; Bowe, P D; Butler, E; Carpenter, P T; Cesar, C L; Chapman, S; Charlton, M; Fajans, J; Friesen, T; Fujiwara, M C; Gill, D R; Hangst, J S; Hardy, W N; Hayden, M E; Humphries, A J; Hurt, J L; Hydomako, R; Jonsell, S; Madsen, N; Menary, S; Nolan, P; Olchanski, K; Olin, A; Povilus, A; Pusa, P; Robicheaux, F; Sarid, E; Silveira, D M; So, C; Storey, J W; Thompson, R I; van der Werf, D P; Wurtele, J S; Yamazaki, Y

    2011-01-14

    We demonstrate controllable excitation of the center-of-mass longitudinal motion of a thermal antiproton plasma using a swept-frequency autoresonant drive. When the plasma is cold, dense, and highly collective in nature, we observe that the entire system behaves as a single-particle nonlinear oscillator, as predicted by a recent theory. In contrast, only a fraction of the antiprotons in a warm plasma can be similarly excited. Antihydrogen was produced and trapped by using this technique to drive antiprotons into a positron plasma, thereby initiating atomic recombination.

  4. Autoresonant Excitation of Antiproton Plasmas

    SciTech Connect

    Andresen, G. B.; Bowe, P. D.; Hangst, J. S.; Ashkezari, M. D.; Hayden, M. E.; Baquero-Ruiz, M.; Chapman, S.; Fajans, J.; Povilus, A.; So, C.; Bertsche, W.; Butler, E.; Charlton, M.; Humphries, A. J.; Madsen, N.; Werf, D. P. van der; Carpenter, P. T.; Hurt, J. L.; Robicheaux, F.; Cesar, C. L.

    2011-01-14

    We demonstrate controllable excitation of the center-of-mass longitudinal motion of a thermal antiproton plasma using a swept-frequency autoresonant drive. When the plasma is cold, dense, and highly collective in nature, we observe that the entire system behaves as a single-particle nonlinear oscillator, as predicted by a recent theory. In contrast, only a fraction of the antiprotons in a warm plasma can be similarly excited. Antihydrogen was produced and trapped by using this technique to drive antiprotons into a positron plasma, thereby initiating atomic recombination.

  5. Directional excitation without breaking reciprocity

    NASA Astrophysics Data System (ADS)

    Ramezani, Hamidreza; Dubois, Marc; Wang, Yuan; Shen, Y. Ron; Zhang, Xiang

    2016-09-01

    We propose a mechanism for directional excitation without breaking reciprocity. This is achieved by embedding an impedance matched parity-time symmetric potential in a three-port system. The amplitude distribution within the gain and loss regions is strongly influenced by the direction of the incoming field. Consequently, the excitation of the third port is contingent on the direction of incidence while transmission in the main channel is immune. Our design improves the four-port directional coupler scheme, as there is no need to implement an anechoic termination to one of the ports.

  6. 46 CFR 111.12-3 - Excitation.

    Code of Federal Regulations, 2013 CFR

    2013-10-01

    ... (incorporated by reference; see 46 CFR 110.10-1), except that those for mobile offshore drilling units must meet... 46 CFR 110.10-1). In particular, no static exciter may be used for excitation of an emergency... REQUIREMENTS Generator Construction and Circuits § 111.12-3 Excitation. In general, excitation must...

  7. 46 CFR 111.12-3 - Excitation.

    Code of Federal Regulations, 2014 CFR

    2014-10-01

    ... (incorporated by reference; see 46 CFR 110.10-1), except that those for mobile offshore drilling units must meet... 46 CFR 110.10-1). In particular, no static exciter may be used for excitation of an emergency... REQUIREMENTS Generator Construction and Circuits § 111.12-3 Excitation. In general, excitation must...

  8. 46 CFR 111.12-3 - Excitation.

    Code of Federal Regulations, 2012 CFR

    2012-10-01

    ... (incorporated by reference; see 46 CFR 110.10-1), except that those for mobile offshore drilling units must meet... 46 CFR 110.10-1). In particular, no static exciter may be used for excitation of an emergency... REQUIREMENTS Generator Construction and Circuits § 111.12-3 Excitation. In general, excitation must...

  9. High-frequency collective excitations in molten and glassy Te studied by inelastic neutron scattering

    SciTech Connect

    Ruiz-Martin, M. D.; Jimenez-Ruiz, M.; Bermejo, F. J.

    2006-03-01

    The spectra of collective excitations of liquid and glassy tellurium have been studied by means of inelastic neutron scattering. Here we report on the dynamics of liquid Te as measured at two different temperatures, just above melting (T{sub m}=723 K) and at {approx}1000 K as well as the glass that is studied at room temperature. Estimates for the velocity of propagating excitations for both temperatures have been obtained from the experimental data, and a contrasting behavior is found with respect to anomalies shown by the adiabatic sound velocity measured by ultrasound methods. The origin of such differences is finally discussed.

  10. Structure of electron tracks in water. 2. Distribution of primary ionizations and excitations in water radiolysis. [accelerated electrons

    SciTech Connect

    Pimblott, S.M.; Mozumder, A. )

    1991-09-19

    A procedure for the calculation of entity-specific ionization and excitation probabilities for water radiolysis at low linear energy transfer (LET) has been developed. The technique pays due attention to the effects of the ionization threshold and the energy dependence of the ionization efficiency. The numbers of primary ionizations and excitations are not directly proportional to the spur energy. At a given spur energy, ionization follows a binomial distribution subject to an energetically possible maximum. The excitation distribution for a spur of given energy and with a given number of ionizations is given by a geometric series. The occurrence probabilities depend upon the cross sections of ionization, excitation, and other inferior processes. Following the low-LET radiolysis of liquid water the most probable spurs contain one ionization, two ionizations, or one ionization and one excitation, while in water vapor they contain either one ionization or one excitation. In liquid water the most probable outcomes for spurs corresponding to the most probable energy loss (22 eV) and to the mean energy loss (38 eV) are one ionization and one excitation, and two ionizations and one excitation, respectively. In the vapor, the most probable energy loss is 14 eV which results in one ionization or one excitation and the mean energy loss is 34 eV for which the spur of maximum probability contains one ionization and two excitations. The total calculated primary yields for low-LET radiolysis are in approximate agreement with experiment in both phases.

  11. Communicating the Excitement of Science

    ScienceCinema

    Michael Turner

    2016-07-12

    In this talk (which will include some exciting science) I will discuss some lessons I have learned about communicating science to scientists (in my own field and others), students, the public, the press, and policy makers in giving 500+ colloquia and seminars, 300+ public lectures and many informal presentations (including cocktail parties).

  12. Collisional excitation of interstellar water

    NASA Technical Reports Server (NTRS)

    Palma, Amedeo; Green, Sheldon; Defrees, D. J.; Mclean, A. D.

    1988-01-01

    Rates for rotational excitation of water molecules in collisions with He atoms have been obtained from a new, accurate theoretical interaction potential. Rates among the lowest 40 ortho levels are given for kinetic temperatures to 1400 K and among the lowest 29 para levels for kinetic temperatures to 800 K.

  13. Launch Excitement with Water Rockets

    ERIC Educational Resources Information Center

    Sanchez, Juan Carlos; Penick, John

    2007-01-01

    Explosions and fires--these are what many students are waiting for in science classes. And when they do occur, students pay attention. While we can't entertain our students with continual mayhem, we can catch their attention and cater to their desires for excitement by saying, "Let's make rockets." In this activity, students make simple, reusable…

  14. Pseudorandom selective excitation in NMR

    NASA Astrophysics Data System (ADS)

    Walls, Jamie D.; Coomes, Alexandra

    2011-09-01

    In this work, average Hamiltonian theory is used to study selective excitation under a series of small flip-angle θ-pulses θ ≪ {π}/{3} applied either periodically [corresponding to the DANTE pulse sequence] or aperiodically to a spin-1/2 system. First, an average Hamiltonian description of the DANTE pulse sequence is developed that is valid for frequencies either at or very far from integer multiples of {1}/{τ}, where τ is the interpulse delay. For aperiodic excitation, a single resonance, νsel, can be selectively excited if the θ-pulse phases are modulated in concert with the interpulse delays. The conditions where average Hamiltonian theory can be accurately applied to describe the dynamics under aperiodic selective pulses, which are referred to as pseudorandom-DANTE or p-DANTE sequences, are similar to those found for the DANTE sequence. Signal averaging over different p-DANTE sequences improves the apparent selectivity at νsel by reducing the excitations at other frequencies. Experimental demonstrations of p-DANTE sequences and comparisons with the theory are presented.

  15. Communicating the Excitement of Science

    SciTech Connect

    Michael Turner

    2009-06-05

    In this talk (which will include some exciting science) I will discuss some lessons I have learned about communicating science to scientists (in my own field and others), students, the public, the press, and policy makers in giving 500+ colloquia and seminars, 300+ public lectures and many informal presentations (including cocktail parties).

  16. Perceptual Load Alters Visual Excitability

    ERIC Educational Resources Information Center

    Carmel, David; Thorne, Jeremy D.; Rees, Geraint; Lavie, Nilli

    2011-01-01

    Increasing perceptual load reduces the processing of visual stimuli outside the focus of attention, but the mechanism underlying these effects remains unclear. Here we tested an account attributing the effects of perceptual load to modulations of visual cortex excitability. In contrast to stimulus competition accounts, which propose that load…

  17. Coherent Nonlinear Terahertz Spectroscopy of Halomethane Liquids

    NASA Astrophysics Data System (ADS)

    Finneran, Ian A.; Welsch, Ralph; Allodi, Marco A.; Miller, Thomas F., III; Blake, Geoffrey

    2016-06-01

    The low-energy terahertz motions of liquids greatly influence their behavior, but are not fully understood. Here, we present results from a recently developed heterodyne-detected Terahertz Kerr Effect (TKE) spectrometer, using an intense picosecond terahertz pump pulse, followed by a weak near-infrared femtosecond probe pulse. In the responses of several halomethane liquids, we find evidence for terahertz intramolecular vibrational coupling and the excitation of intermolecular motions. The experimental results are further supported by reduced density matrix and molecular dynamics simulations. With modest improvements in sensitivity, we expect this technique to be applicable to hydrogen-bonded liquids and amorphous solids.

  18. Velocity-modulation atomization of liquid jets

    NASA Technical Reports Server (NTRS)

    Dressler, John L.

    1994-01-01

    A novel atomizer based on high-amplitude velocity atomization has been developed. Presently, the most common methods of atomization can use only the Rayleigh instability of a liquid cylinder and the Kelvin-Helmholtz instability of a liquid sheet. Our atomizer is capable of atomizing liquid jets by the excitation and destabilization of many other higher-order modes of surface deformation. The potential benefits of this sprayer are more uniform fuel air mixtures, faster fuel-air mixing, extended flow ranges for commercial nozzles, and the reduction of nozzle plugging by producing small drops from large nozzles.

  19. Fractionalized spin-wave continuum in kagome spin liquids

    NASA Astrophysics Data System (ADS)

    Mei, Jia-Wei; Wen, Xiao-Gang

    Motivated by spin-wave continuum (SWC) observed in recent neutron scattering experiments in Herbertsmithite, we use Gutzwiller-projected wave functions to study dynamic spin structure factor S (q , ω) of spin liquid states on the kagome lattice. Spin-1 excited states in spin liquids are represented by Gutzwiller-projected two-spinon excited wave functions. We investigate three different spin liquid candidates, spinon Fermi-surface spin liquid (FSL), Dirac spin liquid (DSL) and random-flux spin liquid (RSL). FSL and RSL have low energy peaks in S (q , ω) at K points in the extended magnetic Brillouin zone, in contrast to experiments where low energy peaks are found at M points. There is no obviuos contradiction between DSL and neutron scattering measurements. Besides a fractionalized spin (i.e. spin-1/2), spinons in DSL carry a fractionalized crystal momentum which is potentially detectable in SWC in the neutron scattering measurements.

  20. Band excitation Kelvin probe force microscopy utilizing photothermal excitation

    SciTech Connect

    Collins, Liam E-mail: liq1@ORNL.gov; Rodriguez, Brian J.; Jesse, Stephen; Balke, Nina; Kalinin, Sergei; Li, Qian E-mail: liq1@ORNL.gov

    2015-03-09

    A multifrequency open loop Kelvin probe force microscopy (KPFM) approach utilizing photothermal as opposed to electrical excitation is developed. Photothermal band excitation (PthBE)-KPFM is implemented here in a grid mode on a model test sample comprising a metal-insulator junction with local charge-patterned regions. Unlike the previously described open loop BE-KPFM, which relies on capacitive actuation of the cantilever, photothermal actuation is shown to be highly sensitive to the electrostatic force gradient even at biases close to the contact potential difference (CPD). PthBE-KPFM is further shown to provide a more localized measurement of true CPD in comparison to the gold standard ambient KPFM approach, amplitude modulated KPFM. Finally, PthBE-KPFM data contain information relating to local dielectric properties and electronic dissipation between tip and sample unattainable using conventional single frequency KPFM approaches.

  1. Chiral Spin-Orbital Liquids with Nodal Lines

    NASA Astrophysics Data System (ADS)

    Natori, W. M. H.; Andrade, E. C.; Miranda, E.; Pereira, R. G.

    2016-07-01

    Strongly correlated materials with strong spin-orbit coupling hold promise for realizing topological phases with fractionalized excitations. Here, we propose a chiral spin-orbital liquid as a stable phase of a realistic model for heavy-element double perovskites. This spin liquid state has Majorana fermion excitations with a gapless spectrum characterized by nodal lines along the edges of the Brillouin zone. We show that the nodal lines are topological defects of a non-Abelian Berry connection and that the system exhibits dispersing surface states. We discuss some experimental signatures of this state and compare them with properties of the spin liquid candidate Ba2YMoO6.

  2. Liquid Helium Acoustic Microscope.

    NASA Astrophysics Data System (ADS)

    Steer, Andrew Paul

    Available from UMI in association with The British Library. In an acoustic microscope, images are generated by monitoring the intensity of the ultrasonic reflection, or echo, from the surface of a sample. In order to achieve this a pulse of acoustic energy is produced by the excitation of a thin film transducer. The pulse thus generated propagates through a crystal and is incident upon the acoustic lens surface, which is the boundary between the crystal and an acoustic coupling liquid. The acoustic lens is a converging element, and brings the ultrasonic beam to a focus within the liquid. A sample, placed at the focus, can act as a reflector, and the returned pulse then contains information regarding the acoustic reflectivity of this specimen. Acoustic pulses are repeatedly launched and detected while the acoustic lens is scanned over the surface of the sample. In this manner an acoustic image is constructed. Acoustic losses in room temperature liquid coupling media represent a considerable source of difficulty in the recovery of acoustic echo signals. At the frequencies of operation required in a microscope which is capable of high resolution, the ultrasonic attenuation is not only large but increases with the square of frequency. In superfluid liquid helium at temperatures below 0.1 K, however, the ultrasonic attenuation becomes negligible. Furthermore, the low sound velocity in liquid helium results in an increase in resolution, since the acoustic wavelength is proportional to velocity. A liquid helium acoustic microscope has been designed and constructed. Details of the various possible detection methods are given, and comparisons are made between them. Measurements of the performance of the system that was adopted are reported. The development of a cooled preamplifier is also described. The variation of reflected signal with object distance has been measured and compared with theoretical predictions. This variation is important in the analysis of acoustic

  3. Liquid marbles.

    PubMed

    Aussillous, P; Quéré, D

    2001-06-21

    The transport of a small amount of liquid on a solid is not a simple process, owing to the nature of the contact between the two phases. Setting a liquid droplet in motion requires non-negligible forces (because the contact-angle hysteresis generates a force opposing the motion), and often results in the deposition of liquid behind the drop. Different methods of levitation-electrostatic, electromagnetic, acoustic, or even simpler aerodynamic techniques-have been proposed to avoid this wetting problem, but all have proved to be rather cumbersome. Here we propose a simple alternative, which consists of encapsulating an aqueous liquid droplet with a hydrophobic powder. The resulting 'liquid marbles' are found to behave like a soft solid, and show dramatically reduced adhesion to a solid surface. As a result, motion can be generated using gravitational, electrical and magnetic fields. Moreover, because the viscous friction associated with motion is very small, we can achieve quick displacements of the droplets without any leaks. All of these features are of potential benefit in microfluidic applications, and also permit the study of a drop in a non-wetting situation-an issue of renewed interest following the recent achievement of super-hydrophobic substrates. PMID:11418851

  4. Liquid marbles.

    PubMed

    Aussillous, P; Quéré, D

    2001-06-21

    The transport of a small amount of liquid on a solid is not a simple process, owing to the nature of the contact between the two phases. Setting a liquid droplet in motion requires non-negligible forces (because the contact-angle hysteresis generates a force opposing the motion), and often results in the deposition of liquid behind the drop. Different methods of levitation-electrostatic, electromagnetic, acoustic, or even simpler aerodynamic techniques-have been proposed to avoid this wetting problem, but all have proved to be rather cumbersome. Here we propose a simple alternative, which consists of encapsulating an aqueous liquid droplet with a hydrophobic powder. The resulting 'liquid marbles' are found to behave like a soft solid, and show dramatically reduced adhesion to a solid surface. As a result, motion can be generated using gravitational, electrical and magnetic fields. Moreover, because the viscous friction associated with motion is very small, we can achieve quick displacements of the droplets without any leaks. All of these features are of potential benefit in microfluidic applications, and also permit the study of a drop in a non-wetting situation-an issue of renewed interest following the recent achievement of super-hydrophobic substrates.

  5. Liquid Crystals

    NASA Technical Reports Server (NTRS)

    1990-01-01

    Thermochromic liquid crystals, or TLCs, are a type of liquid crystals that react to changes in temperature by changing color. The Hallcrest/NASA collaboration involved development of a new way to visualize boundary layer transition in flight and in wind tunnel testing of aircraft wing and body surfaces. TLCs offered a new and potentially better method of visualizing the boundary layer transition in flight. Hallcrest provided a liquid crystal formulation technique that afforded great control over the sensitivity of the liquid crystals to varying conditions. Method is of great use to industry, government and universities for aerodynamic and hydrodynamic testing. Company's principal line is temperature indicating devices for industrial use, such as non-destructive testing and flaw detection in electric/electronic systems, medical application, such as diagnostic systems, for retail sale, such as room, refrigerator, baby bath and aquarium thermometers, and for advertising and promotion specials. Additionally, Hallcrest manufactures TLC mixtures for cosmetic applications, and liquid crystal battery tester for Duracell batteries.

  6. Aspects of data on the breakup of highly excited nuclei

    SciTech Connect

    Warwick, A.I.; Wieman, H.H.; Gutbrod, H.H.; Ritter, H.G.; Stelzer, H.; Weik, F.; Kaufman, S.B.; Steinberg, E.P.; Wilkins, B.D.

    1983-05-01

    There is an awakening of theoretical interest in the mechanisms by which nuclear fragments (4 less than or equal to A less than or equal to 150) are produced in violent collisions of heavy ions. With this in mind we review some aspects of the available experimental data and point out some challenging features against which to test the models. The concept of evaporation is tremendously powerful when applied to pieces of nuclei of low excitation (1 or 2 MeV/u). Current interest focuses on higher excitations, at the point where the binding energy of the system vanishes. This is the transition from liquid nuclei to a gas of nucleons, and it may be that the critical phenomena that certainly exist in infinite nuclear matter will be manifest in finite nuclei under these conditions.

  7. Vacuum ultraviolet electronic properties of liquids

    SciTech Connect

    Painter, L.R.

    1989-01-01

    The principal aim of this program has been to study the electronic structure of insulating liquids of biological interest over a broad energy range from 0 to 30 eV. The studies basically consist of measuring the reflectance, transmittance, photoemission and photoionization of dielectric liquids in the vacuum ultraviolet spectral region as a function of angle of incidence and energy. these in turn may be interpreted in terms of the electronic structure of each liquid as it is excited by the passage of a charged particle. Optical data provides indirect evidence that collective effects occur in liquids. Direct observation of their existence is substantiated in studies of the energy distribution of electrons specularly scattered from the liquid surface.

  8. Two-component Fermi-liquid theory - Equilibrium properties of liquid metallic hydrogen

    NASA Technical Reports Server (NTRS)

    Oliva, J.; Ashcroft, N. W.

    1981-01-01

    It is reported that the transition of condensed hydrogen from an insulating molecular crystal phase to a metallic liquid phase, at zero temperature and high pressure, appears possible. Liquid metallic hydrogen (LMH), comprising interpenetrating proton and electron fluids, would constitute a two-component Fermi liquid with both a very high component-mass ratio and long-range, species-dependent bare interactions. The low-temperature equilibrium properties of LMH are examined by means of a generalization to the case of two components of the phenomenological Landau Fermi-liquid theory, and the low-temperature specific heat, compressibility, thermal expansion coefficient and spin susceptibility are given. It is found that the specific heat and the thermal expansion coefficient are vastly greater in the liquid than in the corresponding solid, due to the presence of proton quasiparticle excitations in the liquid.

  9. Dipole excitations in 96Ru

    NASA Astrophysics Data System (ADS)

    Linnemann, A.; Fransen, C.; Gorska, M.; Jolie, J.; Kneissl, U.; Knoch, P.; Mücher, D.; Pitz, H. H.; Scheck, M.; Scholl, C.; Brentano, P. Von

    2005-12-01

    Candidates for the two-phonon quadrupole-octupole 1- state and the two-phonon mixed-symmetry 1+ms state have been identified in the N=52 isotope 96Ru using the nuclear resonance fluorescence technique at the bremsstrahlung facility of the Stuttgart Dynamitron accelerator. Detailed information on energies, spins, branching ratios, and transition strengths of four new dipole excitations in 96Ru have been obtained. The observed dipole excitations are nearly at the same energies as in 94Mo, and the transition probabilities are comparable to those for the decay of the (2+1⊗3-1)1- and the (2+1⊗2+ms)1+ms states in 94Mo.

  10. Excitation energies from ensemble DFT

    NASA Astrophysics Data System (ADS)

    Borgoo, Alex; Teale, Andy M.; Helgaker, Trygve

    2015-12-01

    We study the evaluation of the Gross-Oliveira-Kohn expression for excitation energies E1-E0=ɛ1-ɛ0+∂E/xc,w[ρ] ∂w | ρ =ρ0. This expression gives the difference between an excitation energy E1 - E0 and the corresponding Kohn-Sham orbital energy difference ɛ1 - ɛ0 as a partial derivative of the exchange-correlation energy of an ensemble of states Exc,w[ρ]. Through Lieb maximisation, on input full-CI density functions, the exchange-correlation energy is evaluated accurately and the partial derivative is evaluated numerically using finite difference. The equality is studied numerically for different geometries of the H2 molecule and different ensemble weights. We explore the adiabatic connection for the ensemble exchange-correlation energy. The latter may prove useful when modelling the unknown weight dependence of the exchange-correlation energy.

  11. Collisional excitation of interstellar cyclopropenylidene

    NASA Technical Reports Server (NTRS)

    Green, Sheldon; Defrees, D. J.; Mclean, A. D.

    1987-01-01

    Theoretical rotational excitation rates were computed for C3H2 in collisions with He atoms at temperatures from 30 to 120 K. The intermolecular forces were obtained from accurate self-consistent field and perturbation theory calculations, and collision dynamics were treated within the infinite-order sudden approximation. The accuracy of the latter was examined by comparing with the more exact coupled states approximation.

  12. Excitation rates of heavy quarks

    NASA Astrophysics Data System (ADS)

    Canal, C. A.; Santangelo, E. M.; Ducati, M. B.

    1985-06-01

    We obtain the production rates for c, b, and t quarks in deep-inelastic neutrino- (antineutrino-) nucleon interactions, in the standard six-quark model with left-handed couplings. The results are obtained with the most recent mixing parameters and we include a comparison between quark parametrizations. The excitations are calculated separately for each flavor, allowing the understanding of the role of threshold effects when considered through different rescaling variables.

  13. Supersonic CO laser with RF excitation

    NASA Astrophysics Data System (ADS)

    von Buelow, H.; Zeyfang, E.

    1993-07-01

    A supersonic CO laser with a maximum output power of 990 W was developed. The gas is excited in a dielectrically stabilized radio-frequency discharge before it is cooled to a temperature of 90 K by the adiabatic expansion in a supersonic nozzle. After extraction of laser power the gas is recompressed by a supersonic diffuser and a Roots-pump system. No liquid nitrogen is needed for the operation of the laser. At a pressure of 500 mbar, the RF discharge could be operated homogeneously with a specific input power of 180 W/cu cm. It could be shown that the length of the discharge region and the distance between the discharge and the supersonic nozzle should be rather short. By this, the vibrational relaxation of the carbon monoxide is reduced and more laser power can be obtained. The laser power can be increased by using a folded resonator system. If the laser is operated at a low Fresnel number by inserting an aperture inside the cavity, a nearly diffraction limited beam quality can be obtained. Using a supersonic nozzle with a low Mach number enables the operation of the diffuser with a high pressure recovery. Thereby the overall system efficiency is increased.

  14. Macromolecular liquids

    SciTech Connect

    Safinya, C.R.; Safran, S.A. ); Pincus, P.A. )

    1990-01-01

    Liquids include a broad range of material systems which are of high scientific and technological interest. Generally speaking, these are partially ordered or disordered phases where the individual molecular species have organized themselves on length scales which are larger than simple fluids, typically between 10 Angstroms and several microns. The specific systems reported on in this book include membranes, microemulsions, micelles, liquid crystals, colloidal suspensions, and polymers. They have a major impact on a broad spectrum of technological industries such as displays, plastics, soap and detergents, chemicals and petroleum, and pharmaceuticals.

  15. Wedding ring shaped excitation coil

    DOEpatents

    MacLennan, Donald A.; Tsai, Peter

    2001-01-01

    A high frequency inductively coupled electrodeless lamp includes an excitation coil with an effective electrical length which is less than one half wavelength of a driving frequency applied thereto, preferably much less. The driving frequency may be greater than 100 MHz and is preferably as high as 915 MHz. Preferably, the excitation coil is configured as a non-helical, semi-cylindrical conductive surface having less than one turn, in the general shape of a wedding ring. At high frequencies, the current in the coil forms two loops which are spaced apart and parallel to each other. Configured appropriately, the coil approximates a Helmholtz configuration. The lamp preferably utilizes an bulb encased in a reflective ceramic cup with a pre-formed aperture defined therethrough. The ceramic cup may include structural features to aid in alignment and/or a flanged face to aid in thermal management. The lamp head is preferably an integrated lamp head comprising a metal matrix composite surrounding an insulating ceramic with the excitation integrally formed on the ceramic. A novel solid-state oscillator preferably provides RF power to the lamp. The oscillator is a single active element device capable of providing over 70 watts of power at over 70% efficiency.

  16. Local Optical Excitations in Metals

    NASA Astrophysics Data System (ADS)

    Gibbs, Laurence Kay Doon

    Core spectra of p('6) (--->) p('5)s excitations of rare gas, halogen, and alkali impurities located on the surface and in the bulk of host alkali and Mg metals are presented. The data were obtained by means of differential reflectance spectroscopy in the energy range 5-20 eV using synchrotron radiation. In striking contrast to the absorption profiles of the pure alkalis, linear redshifted profiles are observed at dilution for rare gas adsorbates on alkali surfaces, for Cs adsorbed on Mg, and for Cs dispersed in bulk Na as an alloy. When Cs is dispersed in bulk K the sharp edge characteristic of the pure alkalis is observed. The spectra of Cs and Rb adsorbates on alkali surfaces mirror these same trends, but retain a distinct atomic character. A central result of the present research is that the linear profile may be associated with strong coupling of the excitation to the conduction electrons. A criterion for strong coupling is given which depends on the degree to which the excited impurity level mixes with the host conduction band. There is not at present any theory which can explain these observations. Spectra of halogen adsorbates on alkali and Mg surfaces are also presented; it is found that the ground configuration of isolated halogen atoms on these surfaces is ionic. All the impurity-metal complexes are studied at high concentration when impurity-impurity interactions are important.

  17. Entanglement entropy of electronic excitations.

    PubMed

    Plasser, Felix

    2016-05-21

    A new perspective into correlation effects in electronically excited states is provided through quantum information theory. The entanglement between the electron and hole quasiparticles is examined, and it is shown that the related entanglement entropy can be computed from the eigenvalue spectrum of the well-known natural transition orbital (NTO) decomposition. Non-vanishing entanglement is obtained whenever more than one NTO pair is involved, i.e., in the case of a multiconfigurational or collective excitation. An important implication is that in the case of entanglement it is not possible to gain a complete description of the state character from the orbitals alone, but more specific analysis methods are required to decode the mutual information between the electron and hole. Moreover, the newly introduced number of entangled states is an important property by itself giving information about excitonic structure. The utility of the formalism is illustrated in the cases of the excited states of two interacting ethylene molecules, the conjugated polymer para-phenylene vinylene, and the naphthalene molecule.

  18. Channelopathies of skeletal muscle excitability

    PubMed Central

    Cannon, Stephen C.

    2016-01-01

    Familial disorders of skeletal muscle excitability were initially described early in the last century and are now known to be caused by mutations of voltage-gated ion channels. The clinical manifestations are often striking, with an inability to relax after voluntary contraction (myotonia) or transient attacks of severe weakness (periodic paralysis). An essential feature of these disorders is fluctuation of symptoms that are strongly impacted by environmental triggers such as exercise, temperature, or serum K+ levels. These phenomena have intrigued physiologists for decades, and in the past 25 years the molecular lesions underlying these disorders have been identified and mechanistic studies are providing insights for therapeutic strategies of disease modification. These familial disorders of muscle fiber excitability are “channelopathies” caused by mutations of a chloride channel (ClC-1), sodium channel (NaV1.4), calcium channel (CaV1.1) and several potassium channels (Kir2.1, Kir2.6, Kir3.4). This review provides a synthesis of the mechanistic connections between functional defects of mutant ion channels, their impact on muscle excitability, how these changes cause clinical phenotypes, and approaches toward therapeutics. PMID:25880512

  19. Synaptic Control of Motoneuronal Excitability

    PubMed Central

    Rekling, Jens C.; Funk, Gregory D.; Bayliss, Douglas A.; Dong, Xiao-Wei; Feldman, Jack L.

    2016-01-01

    Movement, the fundamental component of behavior and the principal extrinsic action of the brain, is produced when skeletal muscles contract and relax in response to patterns of action potentials generated by motoneurons. The processes that determine the firing behavior of motoneurons are therefore important in understanding the transformation of neural activity to motor behavior. Here, we review recent studies on the control of motoneuronal excitability, focusing on synaptic and cellular properties. We first present a background description of motoneurons: their development, anatomical organization, and membrane properties, both passive and active. We then describe the general anatomical organization of synaptic input to motoneurons, followed by a description of the major transmitter systems that affect motoneuronal excitability, including ligands, receptor distribution, pre- and postsynaptic actions, signal transduction, and functional role. Glutamate is the main excitatory, and GABA and glycine are the main inhibitory transmitters acting through ionotropic receptors. These amino acids signal the principal motor commands from peripheral, spinal, and supraspinal structures. Amines, such as serotonin and norepinephrine, and neuropeptides, as well as the glutamate and GABA acting at metabotropic receptors, modulate motoneuronal excitability through pre- and postsynaptic actions. Acting principally via second messenger systems, their actions converge on common effectors, e.g., leak K+ current, cationic inward current, hyperpolarization-activated inward current, Ca2+ channels, or presynaptic release processes. Together, these numerous inputs mediate and modify incoming motor commands, ultimately generating the coordinated firing patterns that underlie muscle contractions during motor behavior. PMID:10747207

  20. Entanglement entropy of electronic excitations

    NASA Astrophysics Data System (ADS)

    Plasser, Felix

    2016-05-01

    A new perspective into correlation effects in electronically excited states is provided through quantum information theory. The entanglement between the electron and hole quasiparticles is examined, and it is shown that the related entanglement entropy can be computed from the eigenvalue spectrum of the well-known natural transition orbital (NTO) decomposition. Non-vanishing entanglement is obtained whenever more than one NTO pair is involved, i.e., in the case of a multiconfigurational or collective excitation. An important implication is that in the case of entanglement it is not possible to gain a complete description of the state character from the orbitals alone, but more specific analysis methods are required to decode the mutual information between the electron and hole. Moreover, the newly introduced number of entangled states is an important property by itself giving information about excitonic structure. The utility of the formalism is illustrated in the cases of the excited states of two interacting ethylene molecules, the conjugated polymer para-phenylene vinylene, and the naphthalene molecule.

  1. Convective Excitation of Internal Waves

    NASA Astrophysics Data System (ADS)

    Lecoanet, Daniel; Le Bars, Michael; Burns, Keaton; Vasil, Geoffrey; Quataert, Eliot; Brown, Benjamin; Oishi, Jeffrey

    2015-11-01

    We will present a joint experimental & computational study of internal wave generation by convection. First we describe an experiment using the peculiar property of water that its density maximum is at 4° C . A tank of water cooled from below and heated from above develops a cold, convective layer near 4° C at the bottom of the tank, adjacent to a hot stably stratified layer at the top of the tank. We simulate this setup in 2D using the open-source Dedalus code (dedalus-project.org). Our simulations show that waves are excited from within the convection zone, opposed to at the interface between the convective and stably stratified regions. Finally, we will present 3D simulations of internal wave excitation by convection in a fully compressible atmosphere with multiple density scaleheights. These simulations provide greater freedom in choosing the thermal equilibrium of the system, and are run at higher Rayleigh number. The simulated waves are then compared to analytic predictions of the bulk excitation model.

  2. Self-excited multifractal dynamics

    NASA Astrophysics Data System (ADS)

    Filimonov, V.; Sornette, D.

    2011-05-01

    We introduce the self-excited multifractal (SEMF) model, defined such that the amplitudes of the increments of the process are expressed as exponentials of a long memory of past increments. The principal novel feature of the model lies in the self-excitation mechanism combined with exponential nonlinearity, i.e. the explicit dependence of future values of the process on past ones. The self-excitation captures the microscopic origin of the emergent endogenous self-organization properties, such as the energy cascade in turbulent flows, the triggering of aftershocks by previous earthquakes and the "reflexive" interactions of financial markets. The SEMF process has all the standard stylized facts found in financial time series, which are robust to the specification of the parameters and the shape of the memory kernel: multifractality, heavy tails of the distribution of increments with intermediate asymptotics, zero correlation of the signed increments and long-range correlation of the squared increments, the asymmetry (called "leverage" effect) of the correlation between increments and absolute value of the increments and statistical asymmetry under time reversal.

  3. Collective hypersonic excitations in strongly multiple scattering colloids.

    PubMed

    Still, T; Gantzounis, G; Kiefer, D; Hellmann, G; Sainidou, R; Fytas, G; Stefanou, N

    2011-04-29

    Unprecedented low-dispersion high-frequency acoustic excitations are observed in dense suspensions of elastically hard colloids. The experimental phononic band structure for SiO(2) particles with different sizes and volume fractions is well represented by rigorous full-elastodynamic multiple-scattering calculations. The slow phonons, which do not relate to particle resonances, are localized in the surrounding liquid medium and stem from coherent multiple scattering that becomes strong in the close-packing regime. Such rich phonon-matter interactions in nanostructures, being still unexplored, can open new opportunities in phononics.

  4. Spectrum of a magnetized strong-leg quantum spin ladder.

    PubMed

    Schmidiger, D; Bouillot, P; Guidi, T; Bewley, R; Kollath, C; Giamarchi, T; Zheludev, A

    2013-09-01

    Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg S=1/2 ladder material (C7H10N)2CuBr4 in its entirety, both in the gapped spin liquid and the magnetic field-induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. Density matrix renormalization group calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field-theoretical predictions but also test the limits of that approach. PMID:25166704

  5. Spurious Excitations in Semiclassical Scattering Theory.

    ERIC Educational Resources Information Center

    Gross, D. H. E.; And Others

    1980-01-01

    Shows how through proper handling of the nonuniform motion of semiclassical coordinates spurious excitation terms are eliminated. An application to the problem of nuclear Coulomb excitation is presented as an example. (HM)

  6. Liquid ventilation

    PubMed Central

    Sarkar, Suman; Paswan, Anil; Prakas, S.

    2014-01-01

    Human have lungs to breathe air and they have no gills to breath liquids like fish. When the surface tension at the air-liquid interface of the lung increases as in acute lung injury, scientists started to think about filling the lung with fluid instead of air to reduce the surface tension and facilitate ventilation. Liquid ventilation (LV) is a technique of mechanical ventilation in which the lungs are insufflated with an oxygenated perfluorochemical liquid rather than an oxygen-containing gas mixture. The use of perfluorochemicals, rather than nitrogen as the inert carrier of oxygen and carbon dioxide offers a number of advantages for the treatment of acute lung injury. In addition, there are non-respiratory applications with expanding potential including pulmonary drug delivery and radiographic imaging. It is well-known that respiratory diseases are one of the most common causes of morbidity and mortality in intensive care unit. During the past few years several new modalities of treatment have been introduced. One of them and probably the most fascinating, is of LV. Partial LV, on which much of the existing research has concentrated, requires partial filling of lungs with perfluorocarbons (PFC's) and ventilation with gas tidal volumes using conventional mechanical ventilators. Various physico-chemical properties of PFC's make them the ideal media. It results in a dramatic improvement in lung compliance and oxygenation and decline in mean airway pressure and oxygen requirements. No long-term side-effect reported. PMID:25886321

  7. An incompressible state of a photo-excited electron gas

    PubMed Central

    Chepelianskii, Alexei D.; Watanabe, Masamitsu; Nasyedkin, Kostyantyn; Kono, Kimitoshi; Konstantinov, Denis

    2015-01-01

    Two-dimensional electrons in a magnetic field can form new states of matter characterized by topological properties and strong electronic correlations as displayed in the integer and fractional quantum Hall states. In these states, the electron liquid displays several spectacular characteristics, which manifest themselves in transport experiments with the quantization of the Hall resistance and a vanishing longitudinal conductivity or in thermodynamic equilibrium when the electron fluid becomes incompressible. Several experiments have reported that dissipationless transport can be achieved even at weak, non-quantizing magnetic fields when the electrons absorb photons at specific energies related to their cyclotron frequency. Here we perform compressibility measurements on electrons on liquid helium demonstrating the formation of an incompressible electronic state under these resonant excitation conditions. This new state provides a striking example of irradiation-induced self-organization in a quantum system. PMID:26007282

  8. Discovering work excitement among navy nurses.

    PubMed

    Savage, S; Simms, L M; Williams, R A; Erbin-Roesemann, M

    1993-01-01

    An interest in what makes work exciting among Navy Nurse Corps officers led to the use of Simms' work excitement data collection protocol in Navy Medical Centers. Significant levels of work excitement were found among Navy nurses when compared to civilian nurses in non-military settings. Overall, results indicated that Navy nurses are excited about the variety, the leadership/management experiences, and the opportunities for teaching and learning--elements that are the very essence of Navy nursing practice. PMID:8345880

  9. Two-photon excitation of aluminium phthalocyanines

    SciTech Connect

    Meshalkin, Yu P; Alfimov, E E; Makukha, V K; Vasil'ev, N E; Denisov, A N; Ogirenko, A P

    1999-12-31

    A demonstration is given of the feasibility of two-photon excitation of aluminium phthalocyanine and of the pharmaceutical preparation 'Fotosens', used in photodynamic therapy. The excitation source was an Nd:YAG laser emitting at the 1064 nm wavelength. The spectra of the two-photon-excited luminescence were obtained and the two-photon absorption cross sections were determined. (lasers in medicine)

  10. Resource Paper: Molecular Excited State Relaxation Processes.

    ERIC Educational Resources Information Center

    Rhodes, William

    1979-01-01

    Develops the concept of oscillatory v dissipative limits as it applies to electronic excited state processes in molecular systems. Main emphasis is placed on the radiative and nonradiative dynamics of the excited state of a molecule prepared by interaction with light or some other excitation source. (BT)

  11. Contact resonance atomic force microscopy imaging in air and water using photothermal excitation

    SciTech Connect

    Kocun, Marta; Labuda, Aleksander; Gannepalli, Anil; Proksch, Roger

    2015-08-15

    Contact Resonance Force Microscopy (CR-FM) is a leading atomic force microscopy technique for measuring viscoelastic nano-mechanical properties. Conventional piezo-excited CR-FM measurements have been limited to imaging in air, since the “forest of peaks” frequency response associated with acoustic excitation methods effectively masks the true cantilever resonance. Using photothermal excitation results in clean contact, resonance spectra that closely match the ideal frequency response of the cantilever, allowing unambiguous and simple resonance frequency and quality factor measurements in air and liquids alike. This extends the capabilities of CR-FM to biologically relevant and other soft samples in liquid environments. We demonstrate CR-FM in air and water on both stiff silicon/titanium samples and softer polystyrene-polyethylene-polypropylene polymer samples with the quantitative moduli having very good agreement between expected and measured values.

  12. Efficiency improvement in the cantilever photothermal excitation method using a photothermal conversion layer.

    PubMed

    Inada, Natsumi; Asakawa, Hitoshi; Kobayashi, Taiki; Fukuma, Takeshi

    2016-01-01

    Photothermal excitation is a cantilever excitation method that enables stable and accurate operation for dynamic-mode AFM measurements. However, the low excitation efficiency of the method has often limited its application in practical studies. In this study, we propose a method for improving the photothermal excitation efficiency by coating cantilever backside surface near its fixed end with colloidal graphite as a photothermal conversion (PTC) layer. The excitation efficiency for a standard cantilever of PPP-NCHAuD with a spring constant of ≈40 N/m and a relatively stiff cantilever of AC55 with a spring constant of ≈140 N/m were improved by 6.1 times and 2.5 times, respectively, by coating with a PTC layer. We experimentally demonstrate high stability of the PTC layer in liquid by AFM imaging of a mica surface with atomic resolution in phosphate buffer saline solution for more than 2 h without any indication of possible contamination from the coating. The proposed method, using a PTC layer made of colloidal graphite, greatly enhances photothermal excitation efficiency even for a relatively stiff cantilever in liquid. PMID:27335733

  13. Atom-Molecule Coherence in a One-Dimensional System

    NASA Astrophysics Data System (ADS)

    Citro, R.; Orignac, E.

    2005-09-01

    We study a model of one-dimensional fermionic atoms with a narrow Feshbach resonance that allows them to bind in pairs to form bosonic molecules. We show that at low energy, a coherence develops between the molecule and fermion Luttinger liquids. At the same time, a gap opens in the spin excitation spectrum. The coherence implies that the order parameters for the molecular Bose-Einstein condensation and the atomic BCS pairing become identical. Moreover, both bosonic and fermionic charge density wave correlations decay exponentially, in contrast with a usual Luttinger liquid. We exhibit a Luther-Emery point where the systems can be described in terms of noninteracting pseudofermions. At this point we discuss the threshold behavior of density-density response functions.

  14. Turbulent swirling jets with excitation

    NASA Technical Reports Server (NTRS)

    Taghavi, Rahmat; Farokhi, Saeed

    1988-01-01

    An existing cold-jet facility at NASA Lewis Research Center was modified to produce swirling flows with controllable initial tangential velocity distribution. Two extreme swirl profiles, i.e., one with solid-body rotation and the other predominated by a free-vortex distribution, were produced at identical swirl number of 0.48. Mean centerline velocity decay characteristics of the solid-body rotation jet flow exhibited classical decay features of a swirling jet with S - 0.48 reported in the literature. However, the predominantly free-vortex distribution case was on the verge of vortex breakdown, a phenomenon associated with the rotating flows of significantly higher swirl numbers, i.e., S sub crit greater than or equal to 0.06. This remarkable result leads to the conclusion that the integrated swirl effect, reflected in the swirl number, is inadequate in describing the mean swirling jet behavior in the near field. The relative size (i.e., diameter) of the vortex core emerging from the nozzle and the corresponding tangential velocity distribution are also controlling factors. Excitability of swirling jets is also investigated by exciting a flow with a swirl number of 0.35 by plane acoustic waves at a constant sound pressure level and at various frequencies. It is observed that the cold swirling jet is excitable by plane waves, and that the instability waves grow about 50 percent less in peak r.m.s. amplitude and saturate further upstream compared to corresponding waves in a jet without swirl having the same axial mass flux. The preferred Strouhal number based on the mass-averaged axial velocity and nozzle exit diameter for both swirling and nonswirling flows is 0.4.

  15. Liquid/liquid heat exchanger

    NASA Technical Reports Server (NTRS)

    Miller, C. G.

    1980-01-01

    Conceptual design for heat exchanger, utilizing two immiscible liquids with dissimilar specific gravities in direct contact, is more efficient mechanism of heat transfer than conventional heat exchangers with walls or membranes. Concept could be adapted for collection of heat from solar or geothermal sources.

  16. Volumetric Light-Field Excitation

    PubMed Central

    Schedl, David C.; Bimber, Oliver

    2016-01-01

    We explain how to concentrate light simultaneously at multiple selected volumetric positions by means of a 4D illumination light field. First, to select target objects, a 4D imaging light field is captured. A light field mask is then computed automatically for this selection to avoid illumination of the remaining areas. With one-photon illumination, simultaneous generation of complex volumetric light patterns becomes possible. As a full light-field can be captured and projected simultaneously at the desired exposure and excitation times, short readout and lighting durations are supported. PMID:27363565

  17. Multiarmed Spirals in Excitable Media

    NASA Astrophysics Data System (ADS)

    Vasiev, Bakthier; Siegert, Florian; Weijer, Cornelis

    1997-03-01

    Numerical studies of the properties of multiarmed spirals show that they can form spontaneously in low excitability media. The maximum number of arms in a multiarmed spiral is proportional to the ratio of the single spiral period to the refractoriness of the medium. Multiarmed spirals are formed due to attraction of single spirals if these spirals rotate in the same direction and their tips are less than one wavelength apart, i.e., a spiral broken not far from its tip can evolve into a 2-armed spiral. We propose this mechanism to be responsible for the formation of multiarmed spirals in mounds of the slime mold Dictyostelium discoideum.

  18. High Frequency Chandler Wobble Excitation

    NASA Astrophysics Data System (ADS)

    Seitz, F.; Stuck, J.; Thomas, M.

    2003-04-01

    Variations of Earth rotation on sub-daily to secular timescales are caused by mass redistributions in the Earth system as a consequence of geophysical processes and gravitational influences. Forced oscillations of polar motion are superposed by free oscillations of the Earth, i.e. the Chandler wobble and the free core nutation. In order to study the interactions between externally induced polar motion and the Earth's free oscillations, a non-linear gyroscopic model has been developed. In most of the former investigations on polar motion, the Chandler wobble is introduced as a damped oscillation with predetermined frequency and amplitude. However, as the effect of rotational deformation is a backcoupling mechanism of polar motion on the Earth's rotational dynamics, both period and amplitude of the Chandler wobble are time-dependent when regarding additional excitations from, e.g., atmospheric or oceanic mass redistributions. The gyroscopic model is free of any explicit information concerning amplitude, phase, and period of free oscillations. The characteristics of the Earth's free oscillation is reproduced by the model from rheological and geometrical parameters and rotational deformation is taken into account. This enables to study the time variable Chandler oscillation when the gyro is forced with atmospheric and oceanic angular momentum from the global atmospheric ECHAM3-T21 general circulation model together with the ocean model for circulation and tides OMCT driven by ECHAM including surface pressure. Besides, mass redistributions in the Earth's body due to gravitational and loading deformations are regarded and external torques exerted by Moon and Sun are considered. The numerical results of the gyro are significantly related with the geodetically observed time series of polar motion published by the IERS. It is shown that the consistent excitation is capable to counteract the damping and thus to maintain the Chandler amplitude. Spectral analyses of the ECHAM

  19. Nucleon resonance excitation with CLAS

    SciTech Connect

    R. De Vita; CLAS Collaboration

    2004-09-01

    The study of the baryon spectrum is a fundamental part of the scientific program in Hall B at Jefferson Laboratory. The so called N* program indeed concerns the measurement of the electromagnetic production of exclusive hadronic final states, with the purpose of extracting information on baryon excited states. CLAS, the CEBAF Large Acceptance Spectrometer, is explicitly designed for conducting a broad experimental program in hadronic physics, using the continuous electron beam provided by the laboratory. An overview of the most recent results is presented.

  20. Volumetric Light-Field Excitation.

    PubMed

    Schedl, David C; Bimber, Oliver

    2016-01-01

    We explain how to concentrate light simultaneously at multiple selected volumetric positions by means of a 4D illumination light field. First, to select target objects, a 4D imaging light field is captured. A light field mask is then computed automatically for this selection to avoid illumination of the remaining areas. With one-photon illumination, simultaneous generation of complex volumetric light patterns becomes possible. As a full light-field can be captured and projected simultaneously at the desired exposure and excitation times, short readout and lighting durations are supported. PMID:27363565

  1. Mechanically-Excited Sessile Drops

    NASA Astrophysics Data System (ADS)

    Chang, Chun-Ti; Bostwick, Joshua; Daniel, Susan; Steen, Paul

    2010-11-01

    The volume and contact-line mobility of a sessile drop determine the frequency response of the drop to mechanical excitation. A useful signature of the drop is its response to a sweep of frequency. At particular frequencies the drop exhibits standing wave patterns of different mode numbers and/or azimuthal, spinning motion. We report observations of the spectrum of standing wave patterns and compare to predictions of a linear stability theory. On the side of application, the results suggest how to tune the pinning-unpinning of a sessile drop in order to maximize its translation.

  2. [Neurosteroids. Neuromodulators of cerebral excitability].

    PubMed

    Calixto González, E; Brailowsky, S

    1998-01-01

    Steroids which are produced by the brain are called neurosteroids, and they are able to modulate neurotransmissions: GABAergic; glutamatergic; glycinergic, and cholinergic (nicotine receptor). These effects are of short latency and duration, and do not implicate the cellular genome. The interaction of these neurosteroids with membrane receptors contribute to the regulation of neuronal excitability, and their study has allowed a better understanding of cognitive, hormonal, and epileptic phenomena as well as the development of new drugs with anxiolytic, antidepressive, anesthetic and anti-epileptic effects. PMID:9658699

  3. Volumetric Light-Field Excitation.

    PubMed

    Schedl, David C; Bimber, Oliver

    2016-07-01

    We explain how to concentrate light simultaneously at multiple selected volumetric positions by means of a 4D illumination light field. First, to select target objects, a 4D imaging light field is captured. A light field mask is then computed automatically for this selection to avoid illumination of the remaining areas. With one-photon illumination, simultaneous generation of complex volumetric light patterns becomes possible. As a full light-field can be captured and projected simultaneously at the desired exposure and excitation times, short readout and lighting durations are supported.

  4. [Neurosteroids. Neuromodulators of cerebral excitability].

    PubMed

    Calixto González, E; Brailowsky, S

    1998-01-01

    Steroids which are produced by the brain are called neurosteroids, and they are able to modulate neurotransmissions: GABAergic; glutamatergic; glycinergic, and cholinergic (nicotine receptor). These effects are of short latency and duration, and do not implicate the cellular genome. The interaction of these neurosteroids with membrane receptors contribute to the regulation of neuronal excitability, and their study has allowed a better understanding of cognitive, hormonal, and epileptic phenomena as well as the development of new drugs with anxiolytic, antidepressive, anesthetic and anti-epileptic effects.

  5. Volumetric Light-Field Excitation

    NASA Astrophysics Data System (ADS)

    Schedl, David C.; Bimber, Oliver

    2016-07-01

    We explain how to concentrate light simultaneously at multiple selected volumetric positions by means of a 4D illumination light field. First, to select target objects, a 4D imaging light field is captured. A light field mask is then computed automatically for this selection to avoid illumination of the remaining areas. With one-photon illumination, simultaneous generation of complex volumetric light patterns becomes possible. As a full light-field can be captured and projected simultaneously at the desired exposure and excitation times, short readout and lighting durations are supported.

  6. Gene circuit designs for noisy excitable dynamics.

    PubMed

    Rué, Pau; Garcia-Ojalvo, Jordi

    2011-05-01

    Certain cellular processes take the form of activity pulses that can be interpreted in terms of noise-driven excitable dynamics. Here we present an overview of different gene circuit architectures that exhibit excitable pulses of protein expression, when subject to molecular noise. Different types of excitable dynamics can occur depending on the bifurcation structure leading to the specific excitable phase-space topology. The bifurcation structure is not, however, linked to a particular circuit architecture. Thus a given gene circuit design can sustain different classes of excitable dynamics depending on the system parameters.

  7. Theoretical studies of electronically excited states

    SciTech Connect

    Besley, Nicholas A.

    2014-10-06

    Time-dependent density functional theory is the most widely used quantum chemical method for studying molecules in electronically excited states. However, excited states can also be computed within Kohn-Sham density functional theory by exploiting methods that converge the self-consistent field equations to give excited state solutions. The usefulness of single reference self-consistent field based approaches for studying excited states is demonstrated by considering the calculation of several types of spectroscopy including the infrared spectroscopy of molecules in an electronically excited state, the rovibrational spectrum of the NO-Ar complex, core electron binding energies and the emission spectroscopy of BODIPY in water.

  8. Peculiarities of collisional excitation transfer with excited screened energy levels of atoms

    SciTech Connect

    Gerasimov, V. A.; Gerasimov, V. V.; Pavlinskiy, A. V.

    2007-09-15

    We report an experimental discovery of deviations from the known regularities in collisional excitation transfer processes for metal atoms. The collisional excitation transfer with excited screened energy levels of thulium and dysprosium atoms is studied. The selecting role of the screening 6s shell in collisional excitation transfer is shown.

  9. Excitation of slosh waves associated with low frequency impulsive reverse gravity acceleration of geyser initiation

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Shyu, K. L.

    1992-01-01

    The objective of the cryogenic fluid management of the spacecraft propulsion system is to develop the technology necessary for acquisition or positioning of liquid and vapor within a tank in reduced gravity to enable liquid outflow or vapor venting. The requirement to settle or to position liquid fuel over the outlet end of the spacecraft propellant tank prior to main engine restart poses a microgravity fluid behavior problem. The purpose of the present study is to investigate the stability of the most efficient technique for propellant resettling through the minimization of propellant usage and weight penalties. In this study slosh wave excitation induced by the resettling flow field activated by 0.1 Hz low frequency, impulsive reverse gravity acceleration, during reorientation with the initiation of geyser for liquid fill levels of 30, 50, 65, 70 and 80 percent, have been studied. Characteristics of slosh waves with various frequencies excited are discussed. Slosh wave excitation shift the fluid mass distribution in the container which impose time dependent variations in spacecraft moment of inertia. This information is important for the spacecraft control during the course of liquid reorientation.

  10. Liquid electrode

    DOEpatents

    Ekechukwu, Amy A.

    1994-01-01

    A dropping electrolyte electrode for use in electrochemical analysis of non-polar sample solutions, such as benzene or cyclohexane. The liquid electrode, preferably an aqueous salt solution immiscible in the sample solution, is introduced into the solution in dropwise fashion from a capillary. The electrolyte is introduced at a known rate, thus, the droplets each have the same volume and surface area. The electrode is used in making standard electrochemical measurements in order to determine properties of non-polar sample solutions.

  11. Dual excitation multiphase electrostatic drive

    SciTech Connect

    Niino, Toshiki; Higuchi, Toshiro |; Egawa, Saku

    1995-12-31

    A novel electrostatic drive technology named Dual Excitation Multiphase Electrostatic Drive (DEMED) was presented. A basic DEMED consisted of two plastic films in which 3-phase parallel electrodes were embedded and was driven by a 3-phase ac excitation to the electrodes. Static characteristics of DEMED were calculated and tested and the results agreed very well. Three prototype motors of DEMED were fabricated using commercially available technique. The first prototype consisted of a single slider and stator and generated a linear motion with a slider`s motion range of about 5mm. It weighed 7g and generated a power of 1.6W and a thrust force of 4.4N. The second prototype consisted of 50 layer stack of linear motors, summing their outputs. It weighed 3.6kg and generated a propulsive force of 310N being powered with boosted commercial 3-phase electricity. The third prototype consisted of a rotor and a stator in which electrodes were arranged radially and generated rotational motion. The maximum power of 36mW was generated by the prototype weighing only 260mg for its rotor and stator. From the results of the numerical calculation, a practical design methodology for the motor was determined. An optimal design for a motor employing currently available material and fabrication techniques is provided as an example. Analyses predict that force generation over the interfacial area between the slider and stator of this motor would be 3,900N/m{sup 2}.

  12. Coulomb excitation of Ga73

    NASA Astrophysics Data System (ADS)

    Diriken, J.; Stefanescu, I.; Balabanski, D.; Blasi, N.; Blazhev, A.; Bree, N.; Cederkäll, J.; Cocolios, T. E.; Davinson, T.; Eberth, J.; Ekström, A.; Fedorov, D. V.; Fedosseev, V. N.; Fraile, L. M.; Franchoo, S.; Georgiev, G.; Gladnishki, K.; Huyse, M.; Ivanov, O. V.; Ivanov, V. S.; Iwanicki, J.; Jolie, J.; Konstantinopoulos, T.; Kröll, Th.; Krücken, R.; Köster, U.; Lagoyannis, A.; Lo Bianco, G.; Maierbeck, P.; Marsh, B. A.; Napiorkowski, P.; Patronis, N.; Pauwels, D.; Reiter, P.; Seliverstov, M.; Sletten, G.; van de Walle, J.; van Duppen, P.; Voulot, D.; Walters, W. B.; Warr, N.; Wenander, F.; Wrzosek, K.

    2010-12-01

    The B(E2;Ii→If) values for transitions in 3171Ga40 and 3173Ga42 were deduced from a Coulomb excitation experiment at the safe energy of 2.95 MeV/nucleon using post-accelerated beams of Ga71,73 at the REX-ISOLDE on-line isotope mass separator facility. The emitted γ rays were detected by the MINIBALL γ-detector array, and B(E2;Ii→If) values were obtained from the yields normalized to the known strength of the 2+→0+ transition in the Sn120 target. The comparison of these new results with the data of less neutron-rich gallium isotopes shows a shift of the E2 collectivity toward lower excitation energy when adding neutrons beyond N=40. This supports conclusions from previous studies of the gallium isotopes, which indicated a structural change in this isotopic chain between N=40 and 42. Combined with recent measurements from collinear laser spectroscopy showing a 1/2- spin and parity for the ground state, the extracted results revealed evidence for a 1/2-,3/2- doublet near the ground state in 3173Ga42 differing by at most 0.8 keV in energy.

  13. New Insights in 4f(12)5d(1) Excited States of Tm(2+) through Excited State Excitation Spectroscopy.

    PubMed

    de Jong, Mathijs; Biner, Daniel; Krämer, Karl W; Barandiarán, Zoila; Seijo, Luis; Meijerink, Andries

    2016-07-21

    Optical excitation of ions or molecules typically leads to an expansion of the equilibrium bond lengths in the excited electronic state. However, for 4f(n-1)5d(1) excited states in lanthanide ions both expansion and contraction relative to the 4f(n) ground state have been reported, depending on the crystal field and nature of the 5d state. To probe the equilibrium distance offset between different 4f(n-1)5d(1) excited states, we report excited state excitation (ESE) spectra for Tm(2+) doped in CsCaBr3 and CsCaCl3 using two-color excited state excitation spectroscopy. The ESE spectra reveal sharp lines at low energies, confirming a similar distance offset for 4f(n-1)5d(t2g)(1) states. At higher energies, broader bands are observed, which indicate the presence of excited states with a different offset. On the basis of ab initio embedded-cluster calculations, the broad bands are assigned to two-photon d-d absorption from the excited state. In this work, we demonstrate that ESE is a powerful spectroscopic tool, giving access to information which cannot be obtained through regular one-photon spectroscopy. PMID:27347766

  14. New Insights in 4f(12)5d(1) Excited States of Tm(2+) through Excited State Excitation Spectroscopy.

    PubMed

    de Jong, Mathijs; Biner, Daniel; Krämer, Karl W; Barandiarán, Zoila; Seijo, Luis; Meijerink, Andries

    2016-07-21

    Optical excitation of ions or molecules typically leads to an expansion of the equilibrium bond lengths in the excited electronic state. However, for 4f(n-1)5d(1) excited states in lanthanide ions both expansion and contraction relative to the 4f(n) ground state have been reported, depending on the crystal field and nature of the 5d state. To probe the equilibrium distance offset between different 4f(n-1)5d(1) excited states, we report excited state excitation (ESE) spectra for Tm(2+) doped in CsCaBr3 and CsCaCl3 using two-color excited state excitation spectroscopy. The ESE spectra reveal sharp lines at low energies, confirming a similar distance offset for 4f(n-1)5d(t2g)(1) states. At higher energies, broader bands are observed, which indicate the presence of excited states with a different offset. On the basis of ab initio embedded-cluster calculations, the broad bands are assigned to two-photon d-d absorption from the excited state. In this work, we demonstrate that ESE is a powerful spectroscopic tool, giving access to information which cannot be obtained through regular one-photon spectroscopy.

  15. Pump for Saturated Liquids

    NASA Technical Reports Server (NTRS)

    Elliott, D. G.

    1986-01-01

    Boiling liquids pumped by device based on proven components. Expanding saturated liquid in nozzle and diverting its phases along separate paths in liquid/vapor separator raises pressure of liquid. Liquid cooled in process. Pump makes it unnecessary to pressurize cryogenic liquids in order to pump them. Problems of introducing noncondensable pressurizing gas avoided.

  16. Contactless Inductive Bubble Detection in a Liquid Metal Flow

    PubMed Central

    Gundrum, Thomas; Büttner, Philipp; Dekdouk, Bachir; Peyton, Anthony; Wondrak, Thomas; Galindo, Vladimir; Eckert, Sven

    2016-01-01

    The detection of bubbles in liquid metals is important for many technical applications. The opaqueness and the high temperature of liquid metals set high demands on the measurement system. The high electrical conductivity of the liquid metal can be exploited for contactless methods based on electromagnetic induction. We will present a measurement system which consists of one excitation coil and a pickup coil system on the opposite sides of the pipe. With this sensor we were able to detect bubbles in a sodium flow inside a stainless steel pipe and bubbles in a column filled with a liquid Gallium alloy. PMID:26751444

  17. Contactless Inductive Bubble Detection in a Liquid Metal Flow.

    PubMed

    Gundrum, Thomas; Büttner, Philipp; Dekdouk, Bachir; Peyton, Anthony; Wondrak, Thomas; Galindo, Vladimir; Eckert, Sven

    2016-01-01

    The detection of bubbles in liquid metals is important for many technical applications. The opaqueness and the high temperature of liquid metals set high demands on the measurement system. The high electrical conductivity of the liquid metal can be exploited for contactless methods based on electromagnetic induction. We will present a measurement system which consists of one excitation coil and a pickup coil system on the opposite sides of the pipe. With this sensor we were able to detect bubbles in a sodium flow inside a stainless steel pipe and bubbles in a column filled with a liquid Gallium alloy. PMID:26751444

  18. Frequency and wavelength prediction of ultrasonic induced liquid surface waves.

    PubMed

    Mahravan, Ehsan; Naderan, Hamid; Damangir, Ebrahim

    2016-12-01

    A theoretical investigation of parametric excitation of liquid free surface by a high frequency sound wave is preformed, using potential flow theory. Pressure and velocity distributions, resembling the sound wave, are applied to the free surface of the liquid. It is found that for impinging wave two distinct capillary frequencies will be excited: One of them is the same as the frequency of the sound wave, and the other is equal to the natural frequency corresponding to a wavenumber equal to the horizontal wavenumber of the sound wave. When the wave propagates in vertical direction, mathematical formulation leads to an equation, which has resonance frequency equal to half of the excitation frequency. This can explain an important contradiction between the frequency and the wavelength of capillary waves in the two cases of normal and inclined interaction of the sound wave and the free surface of the liquid.

  19. Frequency and wavelength prediction of ultrasonic induced liquid surface waves.

    PubMed

    Mahravan, Ehsan; Naderan, Hamid; Damangir, Ebrahim

    2016-12-01

    A theoretical investigation of parametric excitation of liquid free surface by a high frequency sound wave is preformed, using potential flow theory. Pressure and velocity distributions, resembling the sound wave, are applied to the free surface of the liquid. It is found that for impinging wave two distinct capillary frequencies will be excited: One of them is the same as the frequency of the sound wave, and the other is equal to the natural frequency corresponding to a wavenumber equal to the horizontal wavenumber of the sound wave. When the wave propagates in vertical direction, mathematical formulation leads to an equation, which has resonance frequency equal to half of the excitation frequency. This can explain an important contradiction between the frequency and the wavelength of capillary waves in the two cases of normal and inclined interaction of the sound wave and the free surface of the liquid. PMID:27566141

  20. Yields of excited states of solutes in irradiated benzene and cyclohexane

    SciTech Connect

    Choi, H.T.; Hirayama, F.; Lipsky, S.

    1984-09-13

    The yields of lowest excited singlet states of diphenyloxazole and p-terphenyl in benzene and of diphenyloxazole, p-terphenyl, and biphenyl in cyclohexane have been measured for excitation by using /sup 85/Kr ..beta.. particles. The dependence of the yield on solute concentration for benzene solutions is shown to be accurately represented by a Stern-Volmer function from 5 x 10/sup -4/ to 10/sup -2/ M and to extrapolate at infinite solute concentration to the yield of excited singlet states of neat liquid benzene. The presence of oxygen in the solution does not affect the extrapolation. The absolute efficiencies of energy transfer from irradiated benzene to the solutes are in good agreement with previous measurements made by using optical excitation below the ionization threshold. These results provide additional confirmation that the mechanism of formation of excited solute states in fast-electron-irradiated benzene does not significantly involve electron or hole capture by the solute. They also demonstrate that the inhomogeneity of energy deposition does not affect the ratio of probabilities of the decay of excited benzene by photon emission to its decay by nonradiative energy transfer to the solute. For cyclohexane solutions, it is confirmed that the yields of excited solute states are lower than in benzene solutions at comparable concentration, but larger than would be expected were the same nonionic mechanism to apply as it does in benzene. The consequences of these conclusions are discussed.

  1. Microwave Excitation In ECRIS plasmas

    SciTech Connect

    Ciavola, G.; Celona, L.; Consoli, F.; Gammino, S.; Maimone, F.; Barbarino, S.; Catalano, R. S.; Mascali, D.; Tumino, L.

    2007-09-28

    A number of phenomena related to the electron cyclotron resonance ion sources (ECRIS) has been better understood recently by means of the improvement of comprehension of the coupling mechanism between microwave generators and ECR plasma. In particular, the two frequency heating and the frequency tuning effect, that permit a remarkable increase of the current for the highest charge states ions, can be explained in terms of modes excitation in the cylindrical cavity of the plasma chamber. Calculations based on this theoretical approach have been performed, and the major results will be presented. It will be shown that the electric field pattern completely changes for a few MHz frequency variations and the changes in ECRIS performances can be correlated to the efficiency of the power transfer between electromagnetic field and plasma.

  2. Coulomb excitation of 107Sn

    NASA Astrophysics Data System (ADS)

    DiJulio, D. D.; Cederkall, J.; Fahlander, C.; Ekström, A.; Hjorth-Jensen, M.; Albers, M.; Bildstein, V.; Blazhev, A.; Darby, I.; Davinson, T.; De Witte, H.; Diriken, J.; Fransen, Ch.; Geibel, K.; Gernhäuser, R.; Görgen, A.; Hess, H.; Iwanicki, J.; Lutter, R.; Reiter, P.; Scheck, M.; Seidlitz, M.; Siem, S.; Taprogge, J.; Tveten, G. M.; Van de Walle, J.; Voulot, D.; Warr, N.; Wenander, F.; Wimmer, K.

    2012-07-01

    The radioactive isotope 107Sn was studied using Coulomb excitation at the REX-ISOLDE facility at CERN. This is the lightest odd-Sn nucleus examined using this technique. The reduced transition probability of the lowest-lying 3/2+ state was measured and is compared to shell-model predictions based on several sets of single-neutron energies relative to 100Sn . Similar to the transition probabilities for the 2+ states in the neutron-deficient even-even Sn nuclei, the measured value is underestimated by shell-model calculations. Part of the strength may be recovered by considering the ordering of the d_{5/2} and g_{7/2} single-neutron states.

  3. Collective excitations of supersymmetric plasma

    SciTech Connect

    Czajka, Alina; Mrowczynski, Stanislaw

    2011-02-15

    Collective excitations of N=1 supersymmetric electromagnetic plasma are studied. Since the Keldysh-Schwinger approach is used, not only equilibrium but also nonequilibrium plasma, which is assumed to be ultrarelativistic, is under consideration. The dispersion equations of photon, photino, electron, and selectron modes are written down and the self-energies, which enter the equations, are computed in the hard loop approximation. The self-energies are discussed in the context of effective action which is also given. The photon modes and electron ones appear to be the same as in the usual ultrarelativistic plasma of electrons, positrons, and photons. The photino modes coincide with the electron ones and the selectron modes are as of a free relativistic massive particle.

  4. Excited Baryons in Holographic QCD

    SciTech Connect

    de Teramond, Guy F.; Brodsky, Stanley J.; /SLAC /Southern Denmark U., CP3-Origins

    2011-11-08

    The light-front holographic QCD approach is used to describe baryon spectroscopy and the systematics of nucleon transition form factors. Baryon spectroscopy and the excitation dynamics of nucleon resonances encoded in the nucleon transition form factors can provide fundamental insight into the strong-coupling dynamics of QCD. The transition from the hard-scattering perturbative domain to the non-perturbative region is sensitive to the detailed dynamics of confined quarks and gluons. Computations of such phenomena from first principles in QCD are clearly very challenging. The most successful theoretical approach thus far has been to quantize QCD on discrete lattices in Euclidean space-time; however, dynamical observables in Minkowski space-time, such as the time-like hadronic form factors are not amenable to Euclidean numerical lattice computations.

  5. Statistical dynamo theory: Mode excitation.

    PubMed

    Hoyng, P

    2009-04-01

    We compute statistical properties of the lowest-order multipole coefficients of the magnetic field generated by a dynamo of arbitrary shape. To this end we expand the field in a complete biorthogonal set of base functions, viz. B= summation operator_{k}a;{k}(t)b;{k}(r) . The properties of these biorthogonal function sets are treated in detail. We consider a linear problem and the statistical properties of the fluid flow are supposed to be given. The turbulent convection may have an arbitrary distribution of spatial scales. The time evolution of the expansion coefficients a;{k} is governed by a stochastic differential equation from which we infer their averages a;{k} , autocorrelation functions a;{k}(t)a;{k *}(t+tau) , and an equation for the cross correlations a;{k}a;{l *} . The eigenfunctions of the dynamo equation (with eigenvalues lambda_{k} ) turn out to be a preferred set in terms of which our results assume their simplest form. The magnetic field of the dynamo is shown to consist of transiently excited eigenmodes whose frequency and coherence time is given by Ilambda_{k} and -1/Rlambda_{k} , respectively. The relative rms excitation level of the eigenmodes, and hence the distribution of magnetic energy over spatial scales, is determined by linear theory. An expression is derived for |a;{k}|;{2}/|a;{0}|;{2} in case the fundamental mode b;{0} has a dominant amplitude, and we outline how this expression may be evaluated. It is estimated that |a;{k}|;{2}/|a;{0}|;{2} approximately 1/N , where N is the number of convective cells in the dynamo. We show that the old problem of a short correlation time (or first-order smoothing approximation) has been partially eliminated. Finally we prove that for a simple statistically steady dynamo with finite resistivity all eigenvalues obey Rlambda_{k}<0 .

  6. Excitation of interstellar hydrogen chloride

    NASA Technical Reports Server (NTRS)

    Neufild, David A.; Green, Sheldon

    1994-01-01

    We have computed new rate coefficients for the collisional excitation of HCl by He, in the close-coupled formalism and using an interaction potential determined recently by Willey, Choong, & DeLucia. Results have been obtained for temperatures between 10 K and 300 K. With the use of the infinite order sudden approximation, we have derived approximate expressions of general applicability which may be used to estimate how the rate constant for a transition (J to J prime) is apportioned among the various hyperfine states F prime of the final state J prime. Using these new rate coefficients, we have obtained predictions for the HCl rotational line strengths expected from a dense clump of interstellar gas, as a function of the HCl fractional abundance. Over a wide range of HCl abundances, we have found that the line luminosities are proportional to abundance(exp 2/3), a general result which can be explained using a simple analytical approximation. Our model for the excitation of HCl within a dense molecular cloud core indicates that the J = 1 goes to 0 line strengths measured by Blake, Keene, & Phillips toward the Orion Molecular Cloud (OMC-1) imply a fractional abundance n(HCl)/n(H2) approximately 2 x 10(exp -9), a value which amounts to only approximately 0.3% of the cosmic abundance of chlorine nuclei. Given a fractional abundance of 2 x 10(exp -9), the contribution of HCl emission to the total radiative cooling of a dense clump is small. For Orion, we predict a flux approximately 10(exp -19) W/sq cm for the HCl J = 3 goes to 2 line near 159.8 micrometers, suggesting that the strength of this line could be measured using the Infrared Space Observatory.

  7. Liquid electrode

    DOEpatents

    Ekechukwu, A.A.

    1994-07-05

    A dropping electrolyte electrode is described for use in electrochemical analysis of non-polar sample solutions, such as benzene or cyclohexane. The liquid electrode, preferably an aqueous salt solution immiscible in the sample solution, is introduced into the solution in dropwise fashion from a capillary. The electrolyte is introduced at a known rate, thus, the droplets each have the same volume and surface area. The electrode is used in making standard electrochemical measurements in order to determine properties of non-polar sample solutions. 2 figures.

  8. Laser-induced separation of hydrogen isotopes in the liquid phase

    DOEpatents

    Freund, Samuel M.; Maier, II, William B.; Beattie, Willard H.; Holland, Redus F.

    1980-01-01

    Hydrogen isotope separation is achieved by either (a) dissolving a hydrogen-bearing feedstock compound in a liquid solvent, or (b) liquefying a hydrogen-bearing feedstock compound, the liquid phase thus resulting being kept at a temperature at which spectral features of the feedstock relating to a particular hydrogen isotope are resolved, i.e., a clear-cut isotope shift is delineated, irradiating the liquid phase with monochromatic radiation of a wavelength which at least preferentially excites those molecules of the feedstock containing a first hydrogen isotope, inducing photochemical reaction in the excited molecules, and separating the reaction product containing the first isotope from the liquid phase.

  9. Measurement of Excited States in {sup 40}Si and Evidence for Weakening of the N=28 Shell Gap

    SciTech Connect

    Campbell, C. M.; Bowen, M. D.; Brown, B. A.; Cook, J. M.; Dinca, D.-C.; Gade, A.; Glasmacher, T.; Starosta, K.; Terry, J. R.; Zwahlen, H.; Aoi, N.; Motobayashi, T.; Sakurai, H.; Takeuchi, S.; Yoneda, K.; Bazin, D.; Mueller, W. F.; Horoi, M.; Kanno, S.; Suzuki, H.

    2006-09-15

    Excited states in {sup 40}Si have been established by detecting {gamma} rays coincident with inelastic scattering and nucleon removal reactions on a liquid hydrogen target. The low excitation energy, 986(5) keV, of the 2{sub 1}{sup +} state provides evidence of a weakening in the N=28 shell closure in a neutron-rich nucleus devoid of deformation-driving proton collectivity.

  10. Circadian regulation of human cortical excitability

    PubMed Central

    Ly, Julien Q. M.; Gaggioni, Giulia; Chellappa, Sarah L.; Papachilleos, Soterios; Brzozowski, Alexandre; Borsu, Chloé; Rosanova, Mario; Sarasso, Simone; Middleton, Benita; Luxen, André; Archer, Simon N.; Phillips, Christophe; Dijk, Derk-Jan; Maquet, Pierre; Massimini, Marcello; Vandewalle, Gilles

    2016-01-01

    Prolonged wakefulness alters cortical excitability, which is essential for proper brain function and cognition. However, besides prior wakefulness, brain function and cognition are also affected by circadian rhythmicity. Whether the regulation of cognition involves a circadian impact on cortical excitability is unknown. Here, we assessed cortical excitability from scalp electroencephalography (EEG) responses to transcranial magnetic stimulation in 22 participants during 29 h of wakefulness under constant conditions. Data reveal robust circadian dynamics of cortical excitability that are strongest in those individuals with highest endocrine markers of circadian amplitude. In addition, the time course of cortical excitability correlates with changes in EEG synchronization and cognitive performance. These results demonstrate that the crucial factor for cortical excitability, and basic brain function in general, is the balance between circadian rhythmicity and sleep need, rather than sleep homoeostasis alone. These findings have implications for clinical applications such as non-invasive brain stimulation in neurorehabilitation. PMID:27339884

  11. Circadian regulation of human cortical excitability.

    PubMed

    Ly, Julien Q M; Gaggioni, Giulia; Chellappa, Sarah L; Papachilleos, Soterios; Brzozowski, Alexandre; Borsu, Chloé; Rosanova, Mario; Sarasso, Simone; Middleton, Benita; Luxen, André; Archer, Simon N; Phillips, Christophe; Dijk, Derk-Jan; Maquet, Pierre; Massimini, Marcello; Vandewalle, Gilles

    2016-06-24

    Prolonged wakefulness alters cortical excitability, which is essential for proper brain function and cognition. However, besides prior wakefulness, brain function and cognition are also affected by circadian rhythmicity. Whether the regulation of cognition involves a circadian impact on cortical excitability is unknown. Here, we assessed cortical excitability from scalp electroencephalography (EEG) responses to transcranial magnetic stimulation in 22 participants during 29 h of wakefulness under constant conditions. Data reveal robust circadian dynamics of cortical excitability that are strongest in those individuals with highest endocrine markers of circadian amplitude. In addition, the time course of cortical excitability correlates with changes in EEG synchronization and cognitive performance. These results demonstrate that the crucial factor for cortical excitability, and basic brain function in general, is the balance between circadian rhythmicity and sleep need, rather than sleep homoeostasis alone. These findings have implications for clinical applications such as non-invasive brain stimulation in neurorehabilitation.

  12. The contribution of electronically excited states to the radiation chemistry of organic systems

    SciTech Connect

    Lipsky, S.

    1992-01-01

    At low concentrations ({le}10{sup {minus}3}M) of aromatic solutes in saturated. hydrocarbon solvents, very efficient transport of electronic energy from photo-excited solvent to aromatic is observed. Effects of temperature, dilution, and quenching additives are being studied. Two-photon pulsed laser excitation gives no evidence of long lived metastable states. The fluorescence quantum yields of saturated hydrocarbon liquids have been studied for excitation wavelengths from 200 to 120 nm. For many compounds, the quantum yields for fluorescence are observed to decline to a minimum value at, or near, previously reported ionization thresholds. At higher energies, the magnitude of the quantum yield for fluorescence begins to increase. Magnetic field effects on intensity of steady-state recombination fluorescence have been observed both for photo-generated and {Beta}{sup {minus}} generated, electron and positive ion geminate pairs in saturated hydrocarbon liquids. The comparison indicates an important contribution . to observed recombination fluorescence from multiple ion-pairs under radiation chemical conditions. For photo-excited aromatic solutes dissolved in saturated hydrocarbon liquids, no magnetic field effect could be observed until surprisingly large excess energies above the threshold for ionization were achieved. This suggests a much smaller average range for the thermalized electron than expected from photoconductivity.

  13. A Hamiltonian approach to the parametric excitation

    NASA Astrophysics Data System (ADS)

    Leroy, V.; Bacri, J.-C.; Hocquet, T.; Devaud, M.

    2006-05-01

    We propose a solution of the parametrically excited oscillator problem using the Hamiltonian formalism introduced by Glauber. The main advantage is that, within the framework of this formalism, the different possible approximations appear much more naturally than in the standard textbook presentation. Experiments on adiabatic and resonant parametric excitations of a pendulum are presented as an illustration, with particular attention being paid to the role played by the phase of the excitation.

  14. The Dynamics of Small Excitable Systems

    NASA Astrophysics Data System (ADS)

    Jung, Peter; Shuai, Jian-Wei

    2005-03-01

    We consider clusters of sodium ion channels similar as found in the nodes of Ranvier in myelinated neurons. The cluster behaves like excitable systems in the limit of large numbers of ion channels. Small clusters of channels, i.e. small excitable systems, exhibit spontaneous action potentials. We show that small excitable systems exhibit maxima of the spontaneous firing rate and of the response to external stimuli at multiple specific cluster sizes that are universally determined by arithmetic properties of small numbers.

  15. Photoionization spectrum of liquid benzene

    SciTech Connect

    Saik, V. O.; Lipsky, S. )

    1994-11-17

    The photocurrent from neat liquid benzene has been studied for excitation energies from threshold to 10.3 eV and for externally applied electric fields from 1 to 50 kV/cm. Using a power law fit to the energy dependence of the threshold current, an onset of [epsilon][sub t] = 7.65 [+-] 0.1 eV has been obtained. The field dependence was fit to an exponential radial probability density for thermalized ion-pair separation distances with an average separation distance of [r] = 23 [+-] 2 A at an excitation energy, [epsilon] of 8.86 eV (1.2 eV above threshold). Photocurrent was too weak to establish a dependence of [r] on excitation energy. The quantum yield for photocurrent at 8.86 eV was determined by comparison with the photocurrent from TMPD in 2,2,4-trimethylpentane (isooctane) to be 6.5 [times] 10[sup [minus]4] at zero field. From this, the intrinsic molecular ionization probability at [epsilon] = 8.86 eV was determined to be 0.6 [+-] 0.3. 30 refs., 5 figs.

  16. Doubly Excited States in Be III

    NASA Astrophysics Data System (ADS)

    Andersen, T.; Bentzen, S. M.; Poulsen, O.

    1980-01-01

    The triplet spectrum of doubly excited Be III has been studied in the wavelength region of 75-5000 Å in order to test the validity of the theoretical term values reported by Lipsky et al. The beam-foil excitation technique was applied to effectively populate the doubly excited states. The identified lower-lying, doubly excited states 2p2 3P, 2pnp 3P, or 3D, and 2pnd 3P, or 3D (n = 3, 4) show that the theoretical term values should be slightly modified.

  17. Two-photon excitation fluorescence bioassays.

    PubMed

    Hänninen, Pekka; Soukka, Jori; Soini, Juhani T

    2008-01-01

    Application of two-photon excitation of fluorescence in microscopy is one of the major discoveries of the "renaissance" of light microscopy that started in the 1980s. The technique derives its advantages from the biologically "smooth" wavelength of the excitation light and the confinement of the excitation. Difficult, and seemingly nontransparent, samples may be imaged with the technique with good resolution. Although the bioresearch has been concentrating mostly on the positive properties of the technique for imaging, the same properties may be applied successfully to nonimaging bioassays. This article focuses on the development path of two-photon excitation-based assay system. PMID:18596366

  18. Laser Excited Fluorescence Studies Of Black Liquor

    NASA Astrophysics Data System (ADS)

    Horvath, J. J.; Semerjian, H. G.

    1986-10-01

    Laser excited fluorescence of black liquor was investigated as a possible monitoring technique for pulping processes. A nitrogen pumped dye laser was used to examine the fluorescence spectrum of black liquor solutions. Various excitation wavelengths were used between 290 and 403 nm. Black liquor fluorescence spectra were found to vary with both excitation wavelength and black liquor concentration. Laser excited fluorescence was found to be a sensitive technique for measurement of black liquor with good detection limits and linear response over a large dynamic range.

  19. Counting Electrons on Liquid Helium

    NASA Astrophysics Data System (ADS)

    Glasson, Phillip

    2004-03-01

    Electrons on liquid helium, localised in an array of quantum dots, have been proposed as condensed matter qubits [M.I.Dykman et al. Phys.Rev. B 67, 155402 (2003)]. The ground and first excited Rydberg states in the vertical potential well on the helium surface would represent |0> and |1>. This requires (a) novel electronic devices on helium using microstructured substrates, (b) excitation of Rydberg states using millimetric microwaves and (c) detection of individual electrons and their quantum states. Progress in meeting these challenges will be presented. An AC-coupled Field Effect Transistor (FET) has been made on GaAs, using free electrons on suspended liquid helium microchannels, 16 micron wide and 1.6 microns deep [P.Glasson et al, Phys.Rev.Lett. 87 176802 (2001)]. The microwave absorption to the first excited Rydberg state near 200 GHz has been measured below 1 K [E.Collin et al. Phys.Rev.Lett. 89, 245301 (2002)], where the temperature-dependent contribution to the linewidth is small. High values of the ratio of the Rabi frequency to the linewidth are obtained. Electrons are trapped on a 5 micron diameter pool of superfluid helium, above a single-electron-transistor (SET) as a detector. The pool is charged from a surface electron reservoir and we count the electrons into and out of the trap. Individual electrons can be stored, detected and counted: the next stage is quantum state detection. The prospects for qubits and quantum information processing with electrons on helium will be assessed.

  20. High Average Power Laser Gain Medium With Low Optical Distortion Using A Transverse Flowing Liquid Host

    DOEpatents

    Comaskey, Brian J.; Ault, Earl R.; Kuklo, Thomas C.

    2005-07-05

    A high average power, low optical distortion laser gain media is based on a flowing liquid media. A diode laser pumping device with tailored irradiance excites the laser active atom, ion or molecule within the liquid media. A laser active component of the liquid media exhibits energy storage times longer than or comparable to the thermal optical response time of the liquid. A circulation system that provides a closed loop for mixing and circulating the lasing liquid into and out of the optical cavity includes a pump, a diffuser, and a heat exchanger. A liquid flow gain cell includes flow straighteners and flow channel compression.

  1. Longitudinal and transverse modes of slosh wave excitation in rotating dewar associated with gravity jitters

    NASA Technical Reports Server (NTRS)

    Hung, R. J.; Lee, C. C.; Leslie, F. W.

    1991-01-01

    Characteristics of slosh waves based on the dynamical behavior of oscillations at the liquid-vapor interface have been investigated. Twelve case studies of slosh wave excitation due to various frequencies of gravity jitters under different rotating speeds of the propellant tank and different levels of background gravity environment have been simulated. The study shows that slosh waves excited inside the spacecraft propellant tank are characterized by the lowest frequency of the waves initiated, frequencies of the gravity jitters imposed on the propellant system, the levels of background gravity environment, and dewar rotating speeds. Conditions for suppression and amplification of the slosh waves are discussed.

  2. Transport currents in Bose quantum liquids

    SciTech Connect

    Apaja, V.; Krotscheck, E.; Rimnac, A.; Zillich, R. E.

    2006-09-07

    Until now, most of what has been said about excitations in quantum liquids has concerned the dynamic structure function, which is observable by means of neutron scattering. The dynamic structure function can be calculated using standard linear response theory. However, at this level one needs only transition densities <0{rho}n> or transition currents <0jn>, which are oscillatory in time and hence do not describe mass transport. In this work we go a step further and study transport currents in excited states, , which requires the calculation of to second order. For that purpose, we take a well-tested microscopic theory of inhomogeneous quantum liquids and extend it to find the currents formed when helium atoms scatter off a helium slab or when excitations evaporate atoms (a setup experimented by A. F. G. Wyatt's group in Exeter). Current conservation was already a major theoretical problem encountered by R. Feynman and led him to introduce backflow corrections. We show that perfect current conservation is expected only for exact solutions of the time-dependent many-body Schroedinger equation. This is the first extensive theoretical study of transport phenomena in a quantum liquid based on an accurate microscopic theory.

  3. Multi-photon excitation microscopy

    PubMed Central

    Diaspro, Alberto; Bianchini, Paolo; Vicidomini, Giuseppe; Faretta, Mario; Ramoino, Paola; Usai, Cesare

    2006-01-01

    Multi-photon excitation (MPE) microscopy plays a growing role among microscopical techniques utilized for studying biological matter. In conjunction with confocal microscopy it can be considered the imaging workhorse of life science laboratories. Its roots can be found in a fundamental work written by Maria Goeppert Mayer more than 70 years ago. Nowadays, 2PE and MPE microscopes are expected to increase their impact in areas such biotechnology, neurobiology, embryology, tissue engineering, materials science where imaging can be coupled to the possibility of using the microscopes in an active way, too. As well, 2PE implementations in noninvasive optical bioscopy or laser-based treatments point out to the relevance in clinical applications. Here we report about some basic aspects related to the phenomenon, implications in three-dimensional imaging microscopy, practical aspects related to design and realization of MPE microscopes, and we only give a list of potential applications and variations on the theme in order to offer a starting point for advancing new applications and developments. PMID:16756664

  4. Multi-photon excitation microscopy.

    PubMed

    Diaspro, Alberto; Bianchini, Paolo; Vicidomini, Giuseppe; Faretta, Mario; Ramoino, Paola; Usai, Cesare

    2006-01-01

    Multi-photon excitation (MPE) microscopy plays a growing role among microscopical techniques utilized for studying biological matter. In conjunction with confocal microscopy it can be considered the imaging workhorse of life science laboratories. Its roots can be found in a fundamental work written by Maria Goeppert Mayer more than 70 years ago. Nowadays, 2PE and MPE microscopes are expected to increase their impact in areas such biotechnology, neurobiology, embryology, tissue engineering, materials science where imaging can be coupled to the possibility of using the microscopes in an active way, too. As well, 2PE implementations in noninvasive optical bioscopy or laser-based treatments point out to the relevance in clinical applications. Here we report about some basic aspects related to the phenomenon, implications in three-dimensional imaging microscopy, practical aspects related to design and realization of MPE microscopes, and we only give a list of potential applications and variations on the theme in order to offer a starting point for advancing new applications and developments.

  5. Multi-photon excitation microscopy.

    PubMed

    Diaspro, Alberto; Bianchini, Paolo; Vicidomini, Giuseppe; Faretta, Mario; Ramoino, Paola; Usai, Cesare

    2006-01-01

    Multi-photon excitation (MPE) microscopy plays a growing role among microscopical techniques utilized for studying biological matter. In conjunction with confocal microscopy it can be considered the imaging workhorse of life science laboratories. Its roots can be found in a fundamental work written by Maria Goeppert Mayer more than 70 years ago. Nowadays, 2PE and MPE microscopes are expected to increase their impact in areas such biotechnology, neurobiology, embryology, tissue engineering, materials science where imaging can be coupled to the possibility of using the microscopes in an active way, too. As well, 2PE implementations in noninvasive optical bioscopy or laser-based treatments point out to the relevance in clinical applications. Here we report about some basic aspects related to the phenomenon, implications in three-dimensional imaging microscopy, practical aspects related to design and realization of MPE microscopes, and we only give a list of potential applications and variations on the theme in order to offer a starting point for advancing new applications and developments. PMID:16756664

  6. Cosmology with liquid mirror telescopes

    NASA Astrophysics Data System (ADS)

    Hogg, David W.; Gibson, Brad K.; Hickson, Paul

    1993-01-01

    Liquid mirrors provide an exciting means to obtain large optical telescopes for substantially lower costs than conventional technologies. The liquid mirror concept has been demonstrated in the lab with the construction of a diffraction limited 1.5 m mirror. The mirror surface, using liquid mercury, forms a perfect parabolic shape when the mirror cell is rotated at a uniform velocity. A liquid mirror must be able to support a heavy mercury load with minimal flexure and have a fundamental resonant frequency that is as high as possible, to suppress the amplitude of surface waves caused by small vibrations transmitted to the mirror. To minimize the transmission of vibrations to the liquid surface, the entire mirror rests on an air bearing. This necessitates the mirror cell being lightweight, due to the limited load capabilities of the air bearing. The mirror components must also have physical characteristics which minimize the effects of thermal expansion with ambient temperature fluctuations in the observatory. In addition, the 2.7 m mirror construction is designed so that the techniques used may be readily extended to the construction of large mirrors. To attain the goals of a lightweight, rigid mirror, a composite laminant construction was used. The mirror consists of a foam core cut to the desired parabolic shape, with an accuracy of a few mm. An aluminum hub serves as an anchor for the foam and skin, and allows precise centering of the mirror on the air bearing and drive system. Several plys of Kevlar, covered in an epoxy matrix, are then applied to the foam. A final layer of pure epoxy is formed by spin casting. This final layer is parabolic to within a fraction of a mm. An aluminum ring bonded to the circumference of the mirror retains the mercury, and incorporates stainless-steel hard-points for the attachment of balance weights.

  7. Coulomb excitation of radioactive {sup 79}Pb

    SciTech Connect

    Lister, C.J.; Blumenthal, D.; Davids, C.N.

    1995-08-01

    The technical challenges expected in experiments with radioactive beams can already be explored by using ions produced in primary reactions. In addition, the re-excitation of these ions by Coulomb excitation allows a sensitive search for collective states that are well above the yrast line. We are building an experiment to study Coulomb excitation of radioactive ions which are separated from beam particles by the Fragment Mass Analyzer. An array of gamma detectors will be mounted at the focal plane to measure the gamma radiation following re-excitation. Five Compton-suppressed Ge detectors and five planar LEPS detectors will be used. The optimum experiment of this type appears to be the study of {sup 79}Rb following the {sup 24}Mg ({sup 58}Ni,3p) reaction. We calculate that about 5 x 10{sup 5} {sup 79}Rb nuclei/second will reach the excitation foil. This rubidium isotope was selected for study as it is strongly produced and is highly deformed, so easily re-excited. The use of a {sup 58}Ni re-excitation foil offers the best yields. After re-excitation the ions will be subsequently transported into a shielded beamdump to prevent the accumulation of activity.

  8. The Excited State Spectrum of QCD

    SciTech Connect

    Robert Edwards

    2010-08-01

    The determination of the highly excited state spectrum of baryons within QCD is a major theoretical and experimental challenge. I will present recent results from lattice QCD that give some indications on the structure of these highly excited states, and outline on-going and future work needed for a full determination of the spectrum, including strong decays.

  9. Vibrationally excited molecular hydrogen near Herschel 36

    SciTech Connect

    Rachford, Brian L.; Snow, Theodore P.; Ross, Teresa L.

    2014-05-10

    We present the first high resolution UV spectra toward Herschel 36, a Trapezium-like system of high-mass stars contained within the Lagoon Nebula (M8, NGC 6523). The spectra reveal extreme rovibrational excitation of molecular hydrogen in material at a single velocity or very small range of velocities, with this component presumably lying near the star system and undergoing fluorescent excitation. The overall H{sub 2} excitation is similar to, but apparently larger than, that seen toward HD 37903 which previously showed the largest vibrationally excited H{sub 2} column densities seen in UV absorption spectra. While the velocities of the highly excited H{sub 2} lines are consistent within each observation, it appears that they underwent a ∼60 km s{sup –1} redshift during the 3.6 yr between observations. In neither case does the velocity of the highly excited material match the velocity of the bulk of the line-of-sight material which appears to mostly be in the foreground of M8. Recent work shows unusually excited CH and CH{sup +} lines and several unusually broad diffuse interstellar bands toward Herschel 36. Along with the H{sub 2} excitation, all of these findings appear to be related to the extreme environment within ∼0.1 pc of the massive young stellar system.

  10. Excitation-scanning hyperspectral imaging microscope.

    PubMed

    Favreau, Peter F; Hernandez, Clarissa; Heaster, Tiffany; Alvarez, Diego F; Rich, Thomas C; Prabhat, Prashant; Leavesley, Silas J

    2014-04-01

    Hyperspectral imaging is a versatile tool that has recently been applied to a variety of biomedical applications, notably live-cell and whole-tissue signaling. Traditional hyperspectral imaging approaches filter the fluorescence emission over a broad wavelength range while exciting at a single band. However, these emission-scanning approaches have shown reduced sensitivity due to light attenuation from spectral filtering. Consequently, emission scanning has limited applicability for time-sensitive studies and photosensitive applications. In this work, we have developed an excitation-scanning hyperspectral imaging microscope that overcomes these limitations by providing high transmission with short acquisition times. This is achieved by filtering the fluorescence excitation rather than the emission. We tested the efficacy of the excitation-scanning microscope in a side-by-side comparison with emission scanning for detection of green fluorescent protein (GFP)-expressing endothelial cells in highly autofluorescent lung tissue. Excitation scanning provided higher signal-to-noise characteristics, as well as shorter acquisition times (300  ms/wavelength band with excitation scanning versus 3  s/wavelength band with emission scanning). Excitation scanning also provided higher delineation of nuclear and cell borders, and increased identification of GFP regions in highly autofluorescent tissue. These results demonstrate excitation scanning has utility in a wide range of time-dependent and photosensitive applications. PMID:24727909

  11. What Gets a Cell Excited? Kinky Curves

    ERIC Educational Resources Information Center

    Kay, Alan R.

    2014-01-01

    Hodgkin and Huxley's (5) revealing the origins of cellular excitability is one of the great triumphs of physiology. In an extraordinarily deft series of papers, they were able to measure the essential electrical characteristics of neurons and synthesize them into a quantitative model that accounts for the excitability of neurons and other…

  12. Excitation of helium ion by positron impact

    SciTech Connect

    Khan, P.; Ghosh, A.S.

    1986-01-01

    Three (1s,2s,2p) and five (1s,2s,2p,3s-bar,3p-bar) -state close-coupling methods have been employed to calculate the n = 2 excitation cross sections of helium ion by positron impact. The effect of pseudostate is found to be very pronounced in the case of 1s-2s excitation.

  13. Study of excited nucleons and their structure

    SciTech Connect

    Burkert, Volker D.

    2014-01-01

    Recent advances in the study of excited nucleons are discussed. Much of the progress has been achieved due to the availability of high precision meson production data in the photoproduction and electroproduction sectors, the development of multi-channel partial wave analysis techniques, and advances in Lattice QCD with predictions of the full excitation spectrum.

  14. Excitation-scanning hyperspectral imaging microscope

    PubMed Central

    Favreau, Peter F.; Hernandez, Clarissa; Heaster, Tiffany; Alvarez, Diego F.; Rich, Thomas C.; Prabhat, Prashant; Leavesley, Silas J.

    2014-01-01

    Abstract. Hyperspectral imaging is a versatile tool that has recently been applied to a variety of biomedical applications, notably live-cell and whole-tissue signaling. Traditional hyperspectral imaging approaches filter the fluorescence emission over a broad wavelength range while exciting at a single band. However, these emission-scanning approaches have shown reduced sensitivity due to light attenuation from spectral filtering. Consequently, emission scanning has limited applicability for time-sensitive studies and photosensitive applications. In this work, we have developed an excitation-scanning hyperspectral imaging microscope that overcomes these limitations by providing high transmission with short acquisition times. This is achieved by filtering the fluorescence excitation rather than the emission. We tested the efficacy of the excitation-scanning microscope in a side-by-side comparison with emission scanning for detection of green fluorescent protein (GFP)-expressing endothelial cells in highly autofluorescent lung tissue. Excitation scanning provided higher signal-to-noise characteristics, as well as shorter acquisition times (300  ms/wavelength band with excitation scanning versus 3  s/wavelength band with emission scanning). Excitation scanning also provided higher delineation of nuclear and cell borders, and increased identification of GFP regions in highly autofluorescent tissue. These results demonstrate excitation scanning has utility in a wide range of time-dependent and photosensitive applications. PMID:24727909

  15. Ensemble density functional theory method correctly describes bond dissociation, excited state electron transfer, and double excitations

    SciTech Connect

    Filatov, Michael; Huix-Rotllant, Miquel; Burghardt, Irene

    2015-05-14

    State-averaged (SA) variants of the spin-restricted ensemble-referenced Kohn-Sham (REKS) method, SA-REKS and state-interaction (SI)-SA-REKS, implement ensemble density functional theory for variationally obtaining excitation energies of molecular systems. In this work, the currently existing version of the SA-REKS method, which included only one excited state into the ensemble averaging, is extended by adding more excited states to the averaged energy functional. A general strategy for extension of the REKS-type methods to larger ensembles of ground and excited states is outlined and implemented in extended versions of the SA-REKS and SI-SA-REKS methods. The newly developed methods are tested in the calculation of several excited states of ground-state multi-reference systems, such as dissociating hydrogen molecule, and excited states of donor–acceptor molecular systems. For hydrogen molecule, the new method correctly reproduces the distance dependence of the lowest excited state energies and describes an avoided crossing between the doubly excited and singly excited states. For bithiophene–perylenediimide stacked complex, the SI-SA-REKS method correctly describes crossing between the locally excited state and the charge transfer excited state and yields vertical excitation energies in good agreement with the ab initio wavefunction methods.

  16. Ensemble density functional theory method correctly describes bond dissociation, excited state electron transfer, and double excitations.

    PubMed

    Filatov, Michael; Huix-Rotllant, Miquel; Burghardt, Irene

    2015-05-14

    State-averaged (SA) variants of the spin-restricted ensemble-referenced Kohn-Sham (REKS) method, SA-REKS and state-interaction (SI)-SA-REKS, implement ensemble density functional theory for variationally obtaining excitation energies of molecular systems. In this work, the currently existing version of the SA-REKS method, which included only one excited state into the ensemble averaging, is extended by adding more excited states to the averaged energy functional. A general strategy for extension of the REKS-type methods to larger ensembles of ground and excited states is outlined and implemented in extended versions of the SA-REKS and SI-SA-REKS methods. The newly developed methods are tested in the calculation of several excited states of ground-state multi-reference systems, such as dissociating hydrogen molecule, and excited states of donor-acceptor molecular systems. For hydrogen molecule, the new method correctly reproduces the distance dependence of the lowest excited state energies and describes an avoided crossing between the doubly excited and singly excited states. For bithiophene-perylenediimide stacked complex, the SI-SA-REKS method correctly describes crossing between the locally excited state and the charge transfer excited state and yields vertical excitation energies in good agreement with the ab initio wavefunction methods.

  17. Liquid Crystal Devices.

    ERIC Educational Resources Information Center

    Bradshaw, Madeline J.

    1983-01-01

    The nature of liquid crystals and several important liquid crystal devices are described. Ideas for practical experiments to illustrate the properties of liquid crystals and their operation in devices are also described. (Author/JN)

  18. Liquid Crystal Inquiries.

    ERIC Educational Resources Information Center

    Marroum, Renata-Maria

    1996-01-01

    Discusses the properties and classification of liquid crystals. Presents a simple experiment that illustrates the structure of liquid crystals and the differences between the various phases liquid crystals can assume. (JRH)

  19. Decoherence and relaxation of a single electron in a one-dimensional conductor

    NASA Astrophysics Data System (ADS)

    Marguerite, A.; Cabart, C.; Wahl, C.; Roussel, B.; Freulon, V.; Ferraro, D.; Grenier, Ch.; Berroir, J.-M.; Plaçais, B.; Jonckheere, T.; Rech, J.; Martin, T.; Degiovanni, P.; Cavanna, A.; Jin, Y.; Fève, G.

    2016-09-01

    We study the decoherence and relaxation of a single elementary electronic excitation propagating in a one-dimensional chiral conductor. Using two-particle interferences in the electronic analog of the Hong-Ou-Mandel experiment, we analyze quantitatively the decoherence scenario of a single electron propagating along a quantum Hall edge channel at filling factor 2. The decoherence results from the emergence of collective neutral excitations induced by Coulomb interaction and leading, in one dimension, to the destruction of the elementary quasiparticle. This study establishes the relevance of electron quantum optics setups to provide stringent tests of strong interaction effects in one-dimensional conductors described by the Luttinger liquids paradigm.

  20. Localization of electrons and excitations

    NASA Astrophysics Data System (ADS)

    Larsson, Sven

    2006-07-01

    Electrons, electron holes, or excitations in finite or infinite 'multimer systems' may be localized or delocalized. In the theory of Hush, localization depends on the ratio Δ/ λ ( Δ/2 = coupling; λ = reorganization energy). The latter theory has been extended to the infinite system [S. Larsson, A. Klimkāns, Mol. Cryst. Liq. Cryst. 355 (2000) 217]. The metal/insulator transition often takes place abruptly as a function of Δ/ λ. It is argued that localization in a system with un-filled bands cannot be determined on the basis of Mott-Hubbard U alone, but depends on the number of accessible valence states, reorganization energy λ and coupling Δ (=2t). In fact U = 0 does not necessarily imply delocalization. The analysis here shows that there are many different situations for an insulator to metal transition. Charge transfer in doped NiO is characterized by Ni 2+ - Ni 3+ exchange while charge transfer in pure NiO is characterized by a disproportionation 2Ni 2+ → Ni + + Ni 3+. In spite of the great differences between these two cases, U has been applied without discrimination to both. The relevant localization parameters appear to be Δ and λ in the first case, with only two oxidation states, and U, Δ and λ in the second case with three oxidation states. The analysis is extended to insulator-metal transitions, giant magnetic resistance (GMR) and high Tc superconductivity (SC). λ and Δ can be determined quite accurately in quantum mechanical calculations involving only one and two monomers, respectively.

  1. Impact of ground- and excited-state aromaticity on cyclopentadiene and silole excitation energies and excited-state polarities.

    PubMed

    Jorner, Kjell; Emanuelsson, Rikard; Dahlstrand, Christian; Tong, Hui; Denisova, Aleksandra V; Ottosson, Henrik

    2014-07-21

    A new qualitative model for estimating the properties of substituted cyclopentadienes and siloles in their lowest ππ* excited states is introduced and confirmed through quantum chemical calculations, and then applied to explain earlier reported experimental excitation energies. According to our model, which is based on excited-state aromaticity and antiaromaticity, siloles and cyclopentadienes are cross-hyperconjugated "aromatic chameleons" that adapt their electronic structures to conform to the various aromaticity rules in different electronic states (Hückel's rule in the π(2) electronic ground state (S0) and Baird's rule in the lowest ππ* excited singlet and triplet states (S1 and T1)). By using pen-and-paper arguments, one can explain polarity changes upon excitation of substituted cyclopentadienes and siloles, and one can tune their lowest excitation energies by combined considerations of ground- and excited-state aromaticity/antiaromaticity effects. Finally, the "aromatic chameleon" model can be extended to other monocyclic compound classes of potential use in organic electronics, thereby providing a unified view of the S0, T1, and S1 states of a range of different cyclic cross-π-conjugated and cross-hyperconjugated compound classes. PMID:25043523

  2. Hyperspectral imaging fluorescence excitation scanning for detecting colorectal cancer: pilot study

    NASA Astrophysics Data System (ADS)

    Leavesley, Silas J.; Wheeler, Mikayla; Lopez, Carmen; Baker, Thomas; Favreau, Peter F.; Rich, Thomas C.; Rider, Paul F.; Boudreaux, Carole W.

    2016-03-01

    Optical spectroscopy and hyperspectral imaging have shown the theoretical potential to discriminate between cancerous and non-cancerous tissue with high sensitivity and specificity. To date, these techniques have not been able to be effectively translated to endoscope platforms. Hyperspectral imaging of the fluorescence excitation spectrum represents a new technology that may be well-suited for endoscopic implementation. However, the feasibility of detecting differences between normal and cancerous mucosa using fluorescence excitation-scanning hyperspectral imaging has not been evaluated. The objective of this pilot study was to evaluate the changes in the fluorescence excitation spectrum of resected specimen pairs of colorectal adenocarcinoma and normal colorectal mucosa. Patients being treated for colorectal adenocarcinoma were enrolled. Representative adenocarcinoma and normal colonic mucosa specimens were collected from each case. Specimens were flash frozen in liquid nitrogen. Adenocarcinoma was confirmed by histologic evaluation of H&E permanent sections. Hyperspectral image data of the fluorescence excitation of adenocarcinoma and surrounding normal tissue were acquired using a custom microscope configuration previously developed in our lab. Results demonstrated consistent spectral differences between normal and cancerous tissues over the fluorescence excitation spectral range of 390-450 nm. We conclude that fluorescence excitation-scanning hyperspectral imaging may offer an alternative approach for differentiating adenocarcinoma and surrounding normal mucosa of the colon. Future work will focus on expanding the number of specimen pairs analyzed and will utilize fresh tissues where possible, as flash freezing and reconstituting tissues may have altered the autofluorescence properties.

  3. REDISTRIBUTOR FOR LIQUID-LIQUID EXTRACTION COLUMNS

    DOEpatents

    Bradley, J.G.

    1957-10-29

    An improved baffle plate construction to intimately mix immiscible liquid solvents for solvent extraction processes in a liquid-liquid pulse column is described. To prevent the light and heavy liquids from forming separate continuous homogeneous vertical channels through sections of the column, a baffle having radially placed rectangular louvers with deflection plates opening upon alternate sides of the baffle is placed in the column, normal to the axis. This improvement substantially completely reduces strippiig losses due to poor mixing.

  4. Liquid annulus

    NASA Technical Reports Server (NTRS)

    Ludewig, Hans

    1991-01-01

    It is shown that the specific impulse varies with the square root of the temperature and inversely with the square root of the molecular weight of the propellant. Typical values for specific impulse corresponding to various rocket concepts are shown. The Liquid Annulus core concept consists of a fuel element which will be arranged in a moderator block. The advantages as seen for the system are: high specific impulse; structural material will all run at low temperature; and lower fission product inventory because of evaporation. It is felt that this concept is worth at least a first look because of the promise of very high specific impulse. Because of the low thrust, one would probably need a cluster of engines. This is not necessarily bad because there would be some redundancy, but because of the low thrust one might have to refuel while running. Depending on the fuel vaporization, material can be included in the uranium that is injected as one is running along.

  5. Thermal excitations of warped membranes

    NASA Astrophysics Data System (ADS)

    Košmrlj, Andrej; Nelson, David R.

    2014-02-01

    We explore thermal fluctuations of thin planar membranes with a frozen spatially varying background metric and a shear modulus. We focus on a special class of D-dimensional "warped membranes" embedded in a d-dimensional space with d ≥D+1 and a preferred height profile characterized by quenched random Gaussian variables {hα(q)}, α =D+1,...,d, in Fourier space with zero mean and a power-law variance hα(q1)hβ(q2)¯˜δα ,βδq1,-q2q1-dh. The case D =2, d =3, with dh=4 could be realized by flash-polymerizing lyotropic smectic liquid crystals. For D 4-ηf(F) (dh<4-ηf(F)), where ηf(F) is the scaling exponent for tethered surfaces with a flat background metric, and the scaling exponents are related through ηu+ηf=dh-D (ηu+2ηf=4-D).

  6. Excitation gap of fractal quantum hall states in graphene

    NASA Astrophysics Data System (ADS)

    Luo, Wenchen; Chakraborty, Tapash

    2016-01-01

    In the presence of a magnetic field and an external periodic potential the Landau level spectrum of a two-dimensional electron gas exhibits a fractal pattern in the energy spectrum which is described as the Hofstadter’s butterfly. In this work, we develop a Hartree-Fock theory to deal with the electron-electron interaction in the Hofstadter’s butterfly state in a finite-size graphene with periodic boundary conditions, where we include both spin and valley degrees of freedom. We then treat the butterfly state as an electron crystal so that we could obtain the order parameters of the crystal in the momentum space and also in an infinite sample. A phase transition between the liquid phase and the fractal crystal phase can be observed. The excitation gaps obtained in the infinite sample is comparable to those in the finite-size study, and agree with a recent experimental observation.

  7. Supersolid structure and excitation spectrum of soft-core bosons in three dimensions

    NASA Astrophysics Data System (ADS)

    Ancilotto, Francesco; Rossi, Maurizio; Toigo, Flavio

    2013-09-01

    By means of a mean-field method, we have studied the zero-temperature structure and excitation spectrum of a three-dimensional soft-core bosonic system for a value of the interaction strength that favors a crystal structure made of atomic nanoclusters arranged with fcc ordering. In addition to the longitudinal and transverse phonon branches expected for a normal crystal, the excitation spectrum shows a soft mode related to the breaking of gauge symmetry, which signals a partial superfluid character of the solid. Additional evidence of supersolidity is provided by the calculation of the superfluid fraction, which shows a first-order drop, from 1 to 0.4, at the liquid-supersolid transition and a monotonic decrease as the interaction strength parameter is increased. The conditions for the coexistence of the supersolid with the homogeneous superfluid are discussed, and the surface tension of a representative solid-liquid interface is calculated.

  8. Seismic excitation by space shuttles

    USGS Publications Warehouse

    Kanamori, H.; Mori, J.; Sturtevant, B.; Anderson, D.L.; Heaton, T.

    1992-01-01

    Shock waves generated by the space shuttles Columbia (August 13, 1989), Atlantis (April 11, 1991) and Discovery (September 18, 1991) on their return to Edwards Air Force Base, California, were recorded by TERRAscope (Caltech's broadband seismic network), the Caltech-U.S.G.S Southern California Seismic Network (SCSN), and the University of Southern California (USC) Los Angeles Basin Seismic Network. The spatial pattern of the arrival times exhibits hyperbolic shock fronts from which the path, velocity and altitude of the space shuttle could be determined. The shock wave was acoustically coupled to the ground, converted to a seismic wave, and recorded clearly at the broadband TERRAscope stations. The acoustic coupling occurred very differently depending on the conditions of the Earth's surface surrounding the station. For a seismic station located on hard bedrock, the shock wave (N wave) was clearly recorded with little distortion. Aside from the N wave, very little acoustic coupling of the shock wave energy to the ground occurred at these sites. The observed N wave record was used to estimate the overpressure of the shock wave accurately; a pressure change of 0.5 to 2.2 mbars was obtained. For a seismic station located close to the ocean or soft sedimentary basins, a significant amount of shock wave energy was transferred to the ground through acoustic coupling of the shock wave and the oceanic Rayleigh wave. A distinct topography such as a mountain range was found effective to couple the shock wave energy to the ground. Shock wave energy was also coupled to the ground very effectively through large man made structures such as high rise buildings and offshore oil drilling platforms. For the space shuttle Columbia, in particular, a distinct pulse having a period of about 2 to 3 seconds was observed, 12.5 s before the shock wave, with a broadband seismograph in Pasadena. This pulse was probably excited by the high rise buildings in downtown Los Angeles which were

  9. Fast Laser Excitation and Ultrahigh Strain-Rate Deformation

    SciTech Connect

    Robert Averback

    2007-06-03

    Phase evolution induced by single or repeated excitation with energetic femtosecond laser pulses is examined. Of primary interest is the solidification behavior of pure metals at deep undercoolings and self-organization in simple eutectic alloys. Time resolved measurements using third harmonic generation (THG) of light and ultrafast electron diffraction (UED) are employed to elucidate several issues related to fast laser excitation, including heat transport by ballistic and diffusional electrons through multilayer films, the dependence of crystallization velocities on materials properties, mechanisms controlling the transport of heat away from the crystal-liquid interface, and the possibility for quenching pure metals, such as Cu, Ni, and Fe, into the amorphous state. Special samples designed to maximize the quenching speed are developed. The properties of such pure metallic glasses, such as glass and crystallization temperatures, will be measured, if such samples are successfully produced. The measurements are complemented by molecular dynamics computer simulations of the solidification process. The second interest of this research is mesoscopic, self-organization of materials under repeated laser melting, with diffusional relaxation between pulses. We select binary alloys that are immiscible in the solid state but miscible in the liquid state, such as Ag-Cu. Femtosecond laser irradiation is employed to induce melting and to vary the melting time over a wide range, from a few ps to hundreds of ps. This enables us to perform critical experimental tests of key theoretical predictions self-organization in alloys under external forcing, in particular the existence of a threshold value of the forced mixing length for patterning to take place.

  10. Increasing average power in medical ultrasonic endoscope imaging system by coded excitation

    NASA Astrophysics Data System (ADS)

    Chen, Xiaodong; Zhou, Hao; Wen, Shijie; Yu, Daoyin

    2008-12-01

    Medical ultrasonic endoscope is the combination of electronic endoscope and ultrasonic sensor technology. Ultrasonic endoscope sends the ultrasonic probe into coelom through biopsy channel of electronic endoscope and rotates it by a micro pre-motor, which requires that the length of ultrasonic probe is no more than 14mm and the diameter is no more than 2.2mm. As a result, the ultrasonic excitation power is very low and it is difficult to obtain a sharp image. In order to increase the energy and SNR of ultrasonic signal, we introduce coded excitation into the ultrasonic imaging system, which is widely used in radar system. Coded excitation uses a long coded pulse to drive ultrasonic transducer, which can increase the average transmitting power accordingly. In this paper, in order to avoid the overlapping between adjacent echo, we used a four-figure Barker code to drive the ultrasonic transducer, which is modulated at the operating frequency of transducer to improve the emission efficiency. The implementation of coded excitation is closely associated with the transient operating characteristic of ultrasonic transducer. In this paper, the transient operating characteristic of ultrasonic transducer excited by a shock pulse δ(t) is firstly analyzed, and then the exciting pulse generated by special ultrasonic transmitting circuit composing of MD1211 and TC6320. In the final part of the paper, we designed an experiment to validate the coded excitation with transducer operating at 5MHz and a glass filled with ultrasonic coupling liquid as the object. Driven by a FPGA, the ultrasonic transmitting circuit output a four-figure Barker excitation pulse modulated at 5MHz, +/-20 voltage and is consistent with the transient operating characteristic of ultrasonic transducer after matched by matching circuit. The reflected echo from glass possesses coded character, which is identical with the simulating result by Matlab. Furthermore, the signal's amplitude is higher.

  11. Slow excited state phototautomerization in 3-hydroxyisoquinoline.

    PubMed

    Joshi, Neeraj Kumar; Arora, Priyanka; Pant, Sanjay; Joshi, Hem Chandra

    2014-06-01

    In the present work we report the spectral and photophysical properties of 3-hydroxyisoquinoline in various protic/aprotic solvents. Our steady state and time resolved fluorescence data indicates that in the monomer form of 3HIQ phototautomerization can take place in the excited state through excited state intramolecular proton, while as per earlier suggestions phototautomerization in 3HIQ occurs in dimer or complex (in the presence of acetic acid) form. Moreover, we find rather slow tautomerization (occurring on the nanosecond scale). It is found that proton transfer occurs both in the ground as well as excited states and is controlled by the polarity of the solvent.

  12. Surface and bulk excitations in condensed matter

    SciTech Connect

    Ritchie, R.H.

    1988-01-01

    In this lecture collective and single-particle electron excitations of solids will be discussed with emphasis on the properties of metallic and semiconducting materials. However, some of the general properties of long-wavelength collective modes to be discussed are valid for insulators as well, and some considerations apply to nuclear excitations such as optical or acoustical phonons, dipolar plasmons, etc. The concept of elementary excitations in solids, pioneered by Bohm and Pines almost 4 decades ago, has proved to be extremely useful in understanding the properties of systems of many particles, especially in respect to the response to the action of external probes. 32 refs., 12 figs.

  13. Pulse Vector-Excitation Speech Encoder

    NASA Technical Reports Server (NTRS)

    Davidson, Grant; Gersho, Allen

    1989-01-01

    Proposed pulse vector-excitation speech encoder (PVXC) encodes analog speech signals into digital representation for transmission or storage at rates below 5 kilobits per second. Produces high quality of reconstructed speech, but with less computation than required by comparable speech-encoding systems. Has some characteristics of multipulse linear predictive coding (MPLPC) and of code-excited linear prediction (CELP). System uses mathematical model of vocal tract in conjunction with set of excitation vectors and perceptually-based error criterion to synthesize natural-sounding speech.

  14. Helicon wave excitation with helical antennas

    SciTech Connect

    Light, M.; Chen, F.F.

    1995-04-01

    Components of the wave magnetic field in a helicon discharge have been measured with a single-turn, coaxial magnetic probe. Left- and right-handed helical antennas, as well as plane-polarized antennas, were used; and the results were compared with the field patterns computed for a nonuniform plasma. The results show that the right-hand circularly polarized mode is preferentially excited with all antennas, even those designed to excite the left-hand mode. For right-hand excitation, the radial amplitude profiles are in excellent agreement with computations. {copyright} {ital 1995} {ital American} {ital Institute} {ital of} {ital Physics}.

  15. Electro-optical parameters in excited states of some spectrally active molecules

    NASA Astrophysics Data System (ADS)

    Benchea, Andreea Celia; Closca, Valentina; Rusu, Cristina Marcela; Morosanu, Cezarina; Dorohoi, Dana Ortansa

    2014-08-01

    The spectral shifts measured in different solvents are expressed as functions of the solvent macroscopic parameters. The value of the correlation coefficient multiplying the functions of electric permittivity was determined by statistical means. The correlation coefficient depends on the electric dipole moment of the spectrally active molecules. The electro-optical parameters in the ground state of the solute molecules can be approximated by molecular modeling. The excited state parameters are usually estimated using the results obtained both by HyperChem Programme and solvatochromic study. The importance of this approximate method is that it offers information about of the excited state of solute molecule for which our measuring possibilities are very restrictive. The information about the excited electronic state is affected by the limits in which the theories of liquid solutions are developed. Our results refer to two molecules of vitamins from B class, namely B3 and B6.

  16. Measurement of optical trapping forces by use of the two-photon-excited fluorescence of microspheres.

    PubMed

    Kachynski, A V; Kuzmin, A N; Pudavar, H E; Kaputa, D S; Cartwright, A N; Prasad, P N

    2003-12-01

    A novel technique for the calibration of laser trapping systems that utilizes two-photon-excited fluorescence of commercial dye-stained microspheres has been demonstrated. The trapping forces as well as the trapping efficiency have been measured for various liquid environments and trapping depths. The trapping efficiency in water was found to decrease with an increase of trapping depths because of the enlargement of the trapping beam waist caused by aberrations of the optical system.

  17. Gluonic Excitations and Experimental Hall-D at Jefferson Lab

    SciTech Connect

    Stevens, Justin

    2014-07-01

    A new tagged photon beam facility is being constructed in experimental Hall-D at Jefferson Lab as a part of the 12 GeV upgrade program. The 9 GeV linearly-polarized photon beam will be produced via coherent Bremsstrahlung using the CEBAF electron beam, incident on a diamond radiator. The GlueX experiment in Hall-D will use this photon beam to search for and study the pattern of gluonic excitations in the meson spectrum produced through photoproduction reactions with a liquid hydrogen target. Recent lattice QCD calculations predict a rich spectrum of hybrid mesons, that are formed by exciting the gluonic field that couples the quarks. A subset of these hybrid mesons are predicted to have exotic quantum numbers which cannot be formed from a simple qq^- pair, and thus provide an ideal laboratory for testing QCD in the confinement regime. In these proceedings the status of the construction and installation of the GlueX detector will be presented, in addition to simulation results for some reactions of interest in hybrid meson searches.

  18. Broadband surface plasmon wave excitation using dispersion engineering.

    PubMed

    Chasnitsky, Michael; Golosovsky, Michael; Davidov, Dan

    2015-11-16

    High sensitivity of surface-plasmon-based sensors stems from the fact that the surface plasmon is a resonance phenomenon. The resonance results from the phase-matching condition when the phase velocity of the surface plasmon wave and of the lateral component of the incident light become equal. We show that this condition can be satisfied simultaneously for many wavelengths. We demonstrate numerically and experimentally that this allows a surface plasmon resonance that extends over a broad wavelength range. We consider two methods of excitation of such broadband surface plasmon resonance: (i) patterning the interface where the surface plasmon propagates and (ii) broadband coupling through dispersion compensation. We demonstrate extremely broadband surface plasmon excitation at the Au-water or Au-air interface that extends through the whole near-infrared range from λ = 1 μm to 3 μm. We show how this broadband surface plasmon can be used for sensitive spectroscopic sensing, in particular for monitoring wetting/dewetting processes such as thin liquid film growth.

  19. Electrokinetics over liquid/liquid interfaces

    NASA Astrophysics Data System (ADS)

    Squires, Todd M.

    2011-11-01

    Since liquid-liquid interfaces flow in response to an applied stress, one might expect electrokinetic flows at liquid-liquid interfaces to be significantly higher than over liquid-solid interfaces. The earliest predictions for the electrophoretic mobility of charged mercury drops - distinct approaches by Frumkin and Levich (1946), and Booth (1951) - differed by O (a /λD) , where a is the radius of the drop and λD is the Debye screening length. Seeking to reconcile this rather striking discrepancy, Levine (1973) showed double-layer polarization to be the key ingredient. Without a physical mechanism by which electrokinetic effects are enhanced, however, it is difficult to know how general the enhancement is - whether it holds only for liquid metal surfaces, or more generally, for all liquid/liquid surfaces. By considering a series of systems in which a planar metal strip is coated with either a liquid metal or liquid dielectric, we show that the central physical mechanism behind the enhancement predicted by Frumkin and Levich (1946) is the presence of an unmatched electrical stress upon the electrolyte-liquid interface, which establishes a Marangoni stress on the droplet surface and drives it into motion. The source of the unbalanced electrokinetic stress on a liquid metal surface is clear - metals represent equipotential surfaces, so no field exists to drive an equal and opposite force on the surface charge. This might suggest that liquid metals represent a unique system, since dielectric liquids can support finite electric fields, which might be expected to exert an electrical stress on the surface charge that balances the electric stress. We demonstrate, however, that electrical and osmotic stresses on relaxed double-layers internal to dielectric liquids precisely cancel, so that internal electrokinetic stresses generally vanish in closed, ideally polarizable liquids. The enhancement for liquid mercury drops can thus be expected quite generally over clean

  20. Quasiparticle breakdown in a quantum spin liquid.

    PubMed

    Stone, Matthew B; Zaliznyak, Igor A; Hong, Tao; Broholm, Collin L; Reich, Daniel H

    2006-03-01

    Much of modern condensed matter physics is understood in terms of elementary excitations, or quasiparticles--fundamental quanta of energy and momentum. Various strongly interacting atomic systems are successfully treated as a collection of quasiparticles with weak or no interactions. However, there are interesting limitations to this description: in some systems the very existence of quasiparticles cannot be taken for granted. Like unstable elementary particles, quasiparticles cannot survive beyond a threshold where certain decay channels become allowed by conservation laws; their spectrum terminates at this threshold. Such quasiparticle breakdown was first predicted for an exotic state of matter--super-fluid 4He at temperatures close to absolute zero, a quantum Bose liquid where zero-point atomic motion precludes crystallization. Here we show, using neutron scattering, that quasiparticle breakdown can also occur in a quantum magnet and, by implication, in other systems with Bose quasiparticles. We have measured spin excitations in a two-dimensional quantum magnet, piperazinium hexachlorodicuprate (PHCC), in which spin-1/2 copper ions form a non-magnetic quantum spin liquid, and find remarkable similarities with excitations in superfluid 4He. We observe a threshold momentum beyond which the quasiparticle peak merges with the two-quasiparticle continuum. It then acquires a finite energy width and becomes indistinguishable from a leading-edge singularity, so that excited states are no longer quasiparticles but occupy a wide band of energy. Our findings have important ramifications for understanding excitations with gapped spectra in many condensed matter systems, ranging from band insulators to high-transition-temperature superconductors.

  1. Quasiparticle breakdown in a quantum spin liquid.

    PubMed

    Stone, Matthew B; Zaliznyak, Igor A; Hong, Tao; Broholm, Collin L; Reich, Daniel H

    2006-03-01

    Much of modern condensed matter physics is understood in terms of elementary excitations, or quasiparticles--fundamental quanta of energy and momentum. Various strongly interacting atomic systems are successfully treated as a collection of quasiparticles with weak or no interactions. However, there are interesting limitations to this description: in some systems the very existence of quasiparticles cannot be taken for granted. Like unstable elementary particles, quasiparticles cannot survive beyond a threshold where certain decay channels become allowed by conservation laws; their spectrum terminates at this threshold. Such quasiparticle breakdown was first predicted for an exotic state of matter--super-fluid 4He at temperatures close to absolute zero, a quantum Bose liquid where zero-point atomic motion precludes crystallization. Here we show, using neutron scattering, that quasiparticle breakdown can also occur in a quantum magnet and, by implication, in other systems with Bose quasiparticles. We have measured spin excitations in a two-dimensional quantum magnet, piperazinium hexachlorodicuprate (PHCC), in which spin-1/2 copper ions form a non-magnetic quantum spin liquid, and find remarkable similarities with excitations in superfluid 4He. We observe a threshold momentum beyond which the quasiparticle peak merges with the two-quasiparticle continuum. It then acquires a finite energy width and becomes indistinguishable from a leading-edge singularity, so that excited states are no longer quasiparticles but occupy a wide band of energy. Our findings have important ramifications for understanding excitations with gapped spectra in many condensed matter systems, ranging from band insulators to high-transition-temperature superconductors. PMID:16525467

  2. Interfacial Phenomena of Magnetic Fluid with Permanent Magnet in a Longitudinally Excited Container

    SciTech Connect

    Sudo, Seiichi; Wakuda, Hirofumi; Yano, Tetsuya

    2008-02-21

    This paper describes the magnetic fluid sloshing in a longitudinally excited container. Liquid responses of magnetic fluid with a permanent magnet in a circular cylindrical container subject to vertical vibration are investigated. Experiments are performed on a vibration- testing system which provided longitudinal excitation. A cylindrical container made with the acrylic plastic is used in the experiment. A permanent magnet is in the state of floating in a magnetic fluid. The disk-shaped and ring-shaped magnets are examined. The different interfacial phenomena from the usual longitudinal liquid sloshing are observed. It is found that the wave motion frequency of magnetic fluid with a disk-shaped magnet in the container subject to vertical vibration is exactly same that of the excitation. In the case of ring-shaped magnet, the first symmetrical mode of one-half subharmonic response is dominant at lower excitation frequencies. The magnetic fluid disintegration of the free surface was also observed by a high-speed video camera system.

  3. Quantum Spin Liquid Emerging from Antiferromagnetic Order by Introducing Disorder.

    PubMed

    Furukawa, T; Miyagawa, K; Itou, T; Ito, M; Taniguchi, H; Saito, M; Iguchi, S; Sasaki, T; Kanoda, K

    2015-08-14

    Quantum spin liquids, which are spin versions of quantum matter, have been sought after in systems with geometrical frustration. We show that disorder drives a classical magnet into a quantum spin liquid through conducting NMR experiments on an organic Mott insulator, κ-(ET)_{2}Cu[N(CN)_{2}]Cl. Antiferromagnetic ordering in the pristine crystal, when irradiated by x rays, disappears. Spin freezing, spin gap, and critical slowing down are not observed, but gapless spin excitations emerge, suggesting a novel role of disorder that brings forth a quantum spin liquid from a classical ordered state. PMID:26317741

  4. Ways of intensifying liquid dispersion in gas flow

    NASA Astrophysics Data System (ADS)

    Bazarov, V. G.

    Ways of intensifying liquid dispersion in gas flow are examined with a view to increasing the efficiency of the existing atomizing nozzles. It is noted that the most economical method of dispersion intensification, without using any additional power, is the excitation of auto-oscillations in liquid and gas flows. Several methods of generating auto-oscillations in commonly used centrifugal nozzles are discussed. Other developments include the spraying of viscous and contaminated fluids in a field of forced pressure, velocity, and vorticity fluctuations, and also gas saturation of liquids prior to spraying in nozzles with porous elements.

  5. Ionic Liquids Database- (ILThermo)

    National Institute of Standards and Technology Data Gateway

    SRD 147 Ionic Liquids Database- (ILThermo) (Web, free access)   IUPAC Ionic Liquids Database, ILThermo, is a free web research tool that allows users worldwide to access an up-to-date data collection from the publications on experimental investigations of thermodynamic, and transport properties of ionic liquids as well as binary and ternary mixtures containing ionic liquids.

  6. Students Excited by Stellar Discovery

    NASA Astrophysics Data System (ADS)

    2011-02-01

    In the constellation of Ophiuchus, above the disk of our Milky Way Galaxy, there lurks a stellar corpse spinning 30 times per second -- an exotic star known as a radio pulsar. This object was unknown until it was discovered last week by three high school students. These students are part of the Pulsar Search Collaboratory (PSC) project, run by the National Radio Astronomy Observatory (NRAO) in Green Bank, WV, and West Virginia University (WVU). The pulsar, which may be a rare kind of neutron star called a recycled pulsar, was discovered independently by Virginia students Alexander Snider and Casey Thompson, on January 20, and a day later by Kentucky student Hannah Mabry. "Every day, I told myself, 'I have to find a pulsar. I better find a pulsar before this class ends,'" said Mabry. When she actually made the discovery, she could barely contain her excitement. "I started screaming and jumping up and down." Thompson was similarly expressive. "After three years of searching, I hadn't found a single thing," he said, "but when I did, I threw my hands up in the air and said, 'Yes!'." Snider said, "It actually feels really neat to be the first person to ever see something like that. It's an uplifting feeling." As part of the PSC, the students analyze real data from NRAO's Robert C. Byrd Green Bank Telescope (GBT) to find pulsars. The students' teachers -- Debra Edwards of Sherando High School, Leah Lorton of James River High School, and Jennifer Carter of Rowan County Senior High School -- all introduced the PSC in their classes, and interested students formed teams to continue the work. Even before the discovery, Mabry simply enjoyed the search. "It just feels like you're actually doing something," she said. "It's a good feeling." Once the pulsar candidate was reported to NRAO, Project Director Rachel Rosen took a look and agreed with the young scientists. A followup observing session was scheduled on the GBT. Snider and Mabry traveled to West Virginia to assist in the

  7. Nonlinear excited waves on the interventricular septum

    NASA Astrophysics Data System (ADS)

    Bekki, Naoaki; Harada, Yoshifumi; Kanai, Hiroshi

    2012-11-01

    Using a novel ultrasonic noninvasive imaging method, we observe some phase singularities in propagating excited waves on a human cardiac interventricular septum (IVS) for a healthy young male. We present a possible physical model explaining one-dimensional dynamics of phase singularities in nonlinearly excited waves on the IVS. We show that at least one of the observed phase singularities in the excited waves on the IVS can be explained by the Bekki-Nozaki hole solution of the complex Ginzburg-Landau equation without any adjustable parameters. We conclude that the complex Ginzburg-Landau equation is such a suitable model for one-dimensional dynamics of cardiac phase singularities in nonlinearly excited waves on the IVS.

  8. Acoustics of Excited Jets: A Historical Perspective

    NASA Technical Reports Server (NTRS)

    Brown, Cliffard A.

    2005-01-01

    The idea that a jet may be excited by external forcing is not new. The first published demonstration of a jet responding to external pressure waves occurred in the mid-1800's. It was not, however, until the 1950's, with the advent of commercial jet aircraft, that interest in the subject greatly increased. Researchers first used excited jets to study the structure of the jet and attempt to determine the nature of the noise sources. The jet actuators of the time limited the range (Reynolds and Mach numbers) of jets that could be excited. As the actuators improved, more realistic jets could be studied. This has led to a better understanding of how jet excitation may be used not only as a research tool to understand the flow properties and noise generation process, but also as a method to control jet noise.

  9. Broadband single-molecule excitation spectroscopy

    PubMed Central

    Piatkowski, Lukasz; Gellings, Esther; van Hulst, Niek F.

    2016-01-01

    Over the past 25 years, single-molecule spectroscopy has developed into a widely used tool in multiple disciplines of science. The diversity of routinely recorded emission spectra does underpin the strength of the single-molecule approach in resolving the heterogeneity and dynamics, otherwise hidden in the ensemble. In early cryogenic studies single molecules were identified by their distinct excitation spectra, yet measuring excitation spectra at room temperature remains challenging. Here we present a broadband Fourier approach that allows rapid recording of excitation spectra of individual molecules under ambient conditions and that is robust against blinking and bleaching. Applying the method we show that the excitation spectra of individual molecules exhibit an extreme distribution of solvatochromic shifts and distinct spectral shapes. Importantly, we demonstrate that the sensitivity and speed of the broadband technique is comparable to that of emission spectroscopy putting both techniques side-by-side in single-molecule spectroscopy. PMID:26794035

  10. Broadband single-molecule excitation spectroscopy

    NASA Astrophysics Data System (ADS)

    Piatkowski, Lukasz; Gellings, Esther; van Hulst, Niek F.

    2016-01-01

    Over the past 25 years, single-molecule spectroscopy has developed into a widely used tool in multiple disciplines of science. The diversity of routinely recorded emission spectra does underpin the strength of the single-molecule approach in resolving the heterogeneity and dynamics, otherwise hidden in the ensemble. In early cryogenic studies single molecules were identified by their distinct excitation spectra, yet measuring excitation spectra at room temperature remains challenging. Here we present a broadband Fourier approach that allows rapid recording of excitation spectra of individual molecules under ambient conditions and that is robust against blinking and bleaching. Applying the method we show that the excitation spectra of individual molecules exhibit an extreme distribution of solvatochromic shifts and distinct spectral shapes. Importantly, we demonstrate that the sensitivity and speed of the broadband technique is comparable to that of emission spectroscopy putting both techniques side-by-side in single-molecule spectroscopy.

  11. Mode Selective Excitation Using Coherent Control Spectroscopy

    SciTech Connect

    Singh, Ajay K.; Konradi, Jakow; Materny, Arnulf; Sarkar, Sisir K.

    2008-11-14

    Femtosecond time-resolved coherent anti-Stokes Raman scattering (fs-CARS) gives access to ultrafast molecular dynamics. However, femtosecond laser pulses are spectrally broad and therefore coherently excite several molecular modes. While the temporal resolution is high, usually no mode-selective excitation is possible. This paper demonstrates the feasibility of selectively exciting specific molecular vibrations in solution phase with shaped fs laser excitation using a feedback-controlled optimization technique guided by an evolutionary algorithm. This approach is also used to obtain molecule-specific CARS spectra from a mixture of different substances. The optimized phase structures of the fs pulses are characterized to get insight into the control process. Possible applications of the spectrum control are discussed.

  12. Geophysical excitation of nutation and geomagnetic jerks

    NASA Astrophysics Data System (ADS)

    Vondrák, Jan; Ron, Cyril

    2014-05-01

    Recently Zinovy Malkin (2013) proposed that the observed changes of Free Core Nutation parameters (phase, amplitude) might be related to geomagnetic jerks (rapid changes of the secular variations of geomagnetic field). We tested this hypothesis and found that if the numerical integration of Brzezinski broad-band Liouville equations of atmospheric/oceanic excitations is re-initialized at the epochs of geomagnetic jerks, the agreement between the integrated and observed celestial pole offsets is improved significantly. This approach however tacitly assumes that the influence of geomagnetic jerks has a stepwise character, which is physically not acceptable. The present study continues in this effort by introducing a simple continuous excitation function (hypothetically due to geomagnetic jerks). The results of numerical integration of atmospheric/oceanic excitations plus this newly introduced excitation are then compared with the observed celestial pole offsets.

  13. The aeronomy of vibrationally excited ozone

    NASA Technical Reports Server (NTRS)

    Frederick, J. E.; Allen, J. E., Jr.

    1980-01-01

    Theoretical calculations show that above 80 km in the earth's atmosphere the production of vibrationally excited ozone by chemical processes leads to number densities which are usually larger than those expected for local thermodynamic equilibrium. Quenching of highly excited molecules produced in O+O2+M, O3+M provided a significant source of the lower lying states above the mesopause while the 9.6 microns emission of O3 (0,0,1) was a major sink. Analysis of available laboratory results implied that reactions involving excited ozone play a significant role in the global ozone balance despite the relatively small abundance of the molecule. However, this effect is implicit in many of the rate coefficients currently used in stratospheric calculations. In the upper mesosphere and lower thermosphere, where the excited state populations differ from those for thermal equilibrium, published reaction rate data are not necessarily applicable to aeronomic calculations.

  14. Hydrogen Bonds in Excited State Proton Transfer

    NASA Astrophysics Data System (ADS)

    Horke, D. A.; Watts, H. M.; Smith, A. D.; Jager, E.; Springate, E.; Alexander, O.; Cacho, C.; Chapman, R. T.; Minns, R. S.

    2016-10-01

    Hydrogen bonding interactions between biological chromophores and their surrounding protein and solvent environment significantly affect the photochemical pathways of the chromophore and its biological function. A common first step in the dynamics of these systems is excited state proton transfer between the noncovalently bound molecules, which stabilizes the system against dissociation and principally alters relaxation pathways. Despite such fundamental importance, studying excited state proton transfer across a hydrogen bond has proven difficult, leaving uncertainties about the mechanism. Through time-resolved photoelectron imaging measurements, we demonstrate how the addition of a single hydrogen bond and the opening of an excited state proton transfer channel dramatically changes the outcome of a photochemical reaction, from rapid dissociation in the isolated chromophore to efficient stabilization and ground state recovery in the hydrogen bonded case, and uncover the mechanism of excited state proton transfer at a hydrogen bond, which follows sequential hydrogen and charge transfer processes.

  15. Universality of the Phonon-Roton Spectrum in Liquids and Superfluidity of 4He

    NASA Astrophysics Data System (ADS)

    Bobrov, Viktor; Trigger, Sergey; Litinski, Daniel

    2016-06-01

    Based on numerous experimental data on inelastic neutron and X-ray scattering in liquids, we assert that the phonon-roton spectrum of collective excitations, predicted by Landau for superfluid helium, is a universal property of the liquid state. We show that the existence of the roton minimum in the spectrum of collective excitations is caused by the short-range order in liquids. Using the virial theorem, we assume that one more branch of excitations should exist in He II, whose energy spectrum differs from the phonon-roton spectrum. Such excitations are associated with the pole of single-particle Green function, which can have a gap at small values of momenta.

  16. Probing the excitation spectrum of polariton condensates

    SciTech Connect

    Wouters, Michiel; Carusotto, Iacopo

    2009-03-15

    We propose a four-wave mixing experiment to probe the elementary excitation spectrum of a nonequilibrium Bose-Einstein condensate of exciton-polaritons under nonresonant pumping. Analytical calculations based on mean-field theory show that this method is able to reveal the characteristic negative energy feature of the Bogoliubov dispersion. Numerical simulations including the finite spatial profile of the excitation laser spot and a weak disorder confirm the practical utility of the method for realistic condensates.

  17. Plasmoelectronics: coupling plasmonic excitation with electron flow.

    PubMed

    Warren, Scott C; Walker, David A; Grzybowski, Bartosz A

    2012-06-19

    Explorations of the coupling of light and charge via localized surface plasmons have led to the discovery that plasmonic excitation can influence macroscopic flows of charge and, conversely, that charging events can change the plasmonic excitation. We discuss recent theory and experiments in the emerging field of plasmoelectronics, with particular emphasis on the application of these materials to challenges in nanotechnology, energy use, and sensing. PMID:22385329

  18. Fast pulsed excitation wiggler or undulator

    DOEpatents

    van Steenbergen, Arie

    1990-01-01

    A fast pulsed excitation, electromagnetic undulator or wiggler, employing geometrically alternating substacks of thin laminations of ferromagnetic material, together with a single turn current loop excitation of the composite assembly, of such shape and configuration that intense, spatially alternating, magnetic fields are generated; for use as a pulsed mode undulator or wiggler radiator, for use in a Free Electron Laser (FEL) type radiation source or, for use in an Inverse Free Electron Laser (IFEL) charged particle accelerator.

  19. Few cycle pulses in semi-holographic Fermi liquid with impurities

    NASA Astrophysics Data System (ADS)

    Belonenko, Mikhail B.; Konobeeva, Natalia N.; Galkina, Elena N.

    2016-03-01

    Special aspects of few cycle pulses propagation in semi-holographic Fermi liquid with impurities are considered in this paper. Green’s function poles which are in charge of excitation states dispersion law of the liquid under consideration were given according to the ADS/CFT correspondence. The impact of both Fermi liquid parameters and its impurities on the few cycle pulse shape was defined.

  20. Quantitative assessment of radiation force effect at the dielectric air-liquid interface

    PubMed Central

    Capeloto, Otávio Augusto; Zanuto, Vitor Santaella; Malacarne, Luis Carlos; Baesso, Mauro Luciano; Lukasievicz, Gustavo Vinicius Bassi; Bialkowski, Stephen Edward; Astrath, Nelson Guilherme Castelli

    2016-01-01

    We induce nanometer-scale surface deformation by exploiting momentum conservation of the interaction between laser light and dielectric liquids. The effect of radiation force at the air-liquid interface is quantitatively assessed for fluids with different density, viscosity and surface tension. The imparted pressure on the liquids by continuous or pulsed laser light excitation is fully described by the Helmholtz electromagnetic force density. PMID:26856622

  1. Chiral Spin-Orbital Liquids with Nodal Lines.

    PubMed

    Natori, W M H; Andrade, E C; Miranda, E; Pereira, R G

    2016-07-01

    Strongly correlated materials with strong spin-orbit coupling hold promise for realizing topological phases with fractionalized excitations. Here, we propose a chiral spin-orbital liquid as a stable phase of a realistic model for heavy-element double perovskites. This spin liquid state has Majorana fermion excitations with a gapless spectrum characterized by nodal lines along the edges of the Brillouin zone. We show that the nodal lines are topological defects of a non-Abelian Berry connection and that the system exhibits dispersing surface states. We discuss some experimental signatures of this state and compare them with properties of the spin liquid candidate Ba_{2}YMoO_{6}. PMID:27419588

  2. Schwinger boson spin-liquid states on square lattice

    NASA Astrophysics Data System (ADS)

    Yang, Xu; Wang, Fa

    2016-07-01

    We study possible spin liquids on square lattice that respect all lattice symmetries and time-reversal symmetry within the framework of Schwinger boson (mean-field) theory. Such spin liquids have spin gap and emergent Z2 gauge field excitations. We classify them by the projective symmetry group method, and find six spin-liquid states that are potentially relevant to the J1-J2 Heisenberg model. The properties of these states are studied under mean-field approximation. Interestingly we find a spin-liquid state that can go through continuous phase transitions to either the Néel magnetic order or magnetic orders of the wave vector at the Brillouin zone edge center. We also discuss the connection between our results and the Abrikosov fermion spin liquids.

  3. Tailoring dye-sensitized upconversion nanoparticle excitation bands towards excitation wavelength selective imaging

    SciTech Connect

    Wu, Xiang; Lee, Hyungseok; Bilsel, Osman; Zhang, Yuanwei; Li, Zhanjun; Chen, Teresa; Liu, Yi; Duan, Chunying; Shen, Jie; Punjabi, Amol; Han, Gang

    2015-01-01

    One of the key roadblocks in UCNP development is its extremely limited choices of excitation wavelengths. We report a generic design to program UCNPs to possess highly tunable dye characteristic excitation bands. Using such distinctive properties, we were able to develop a new excitation wavelength selective security imaging. Finally, this work unleashed the greater freedom of the excitation wavelengths of the upconversion nanoparticles and we believe it is a game-changer in the field and this method will enable numerous applications that are currently limited by existing UCNPs.

  4. Tailoring Dye-sensitized Upconversion Nanoparticles Excitation Bands towards Excitation Wavelength Selective Imaging

    PubMed Central

    Wu, Xiang; Lee, Hyungseok; Bilsel, Osman; Zhang, Yuanwei; Li, Zhanjun; Chen, Teresa; Liu, Yi; Duan, Chunying; Shen, Jie; Punjabi, Amol; Han, Gang

    2015-01-01

    One of key roadblocks in UCNP development is its extremely limited choices of excitation wavelengths. We report a generic design to program UCNPs to possess highly tunable dye characteristic excitation bands. Using such distinctive properties, we were able to develop a new excitation wavelength selective security imaging. This work unleashed the greater freedom of the excitation wavelengths of the upconversion nanoparticles and we believe it is a game-changer in the field and this method will enable numerous applications that are currently limited by existing UCNPs. PMID:26499208

  5. Excited-State Proton Transfer in Resveratrol and Proposed Mechanism for Plant Resistance to Fungal Infection.

    PubMed

    Simkovitch, Ron; Huppert, Dan

    2015-09-01

    Steady-state and time-resolved fluorescence techniques were employed to study the photophysics and photochemistry of trans-resveratrol. trans-Resveratrol is found in large quantities in fungi-infected grapevine-leaf tissue and plays a direct role in the resistance to plant disease. We found that trans-resveratrol in liquid solution undergoes a trans-cis isomerization process in the excited state at a rate that depends partially on the solvent viscosity, as was found in previous studies on trans-stilbene. The hydroxyl groups of the phenol moieties in resveratrol are weak photoacids. In water and methanol solutions containing weak bases such as acetate, a proton is transferred to the base within the lifetime of the excited state. When resveratrol is adsorbed on cellulose (also a component of the plant's cell wall), the cis-trans process is slow and the lifetime of the excited state increases from several tens of picoseconds in ethanol to about 1.5 ns. Excited-state proton transfer occurs when resveratrol is adsorbed on cellulose and acetate ions are in close proximity to the phenol moieties. We propose that proton transfer from excited resveratrol to the fungus acid-sensing chemoreceptor is one of the plant's resistance mechanisms to fungal infection.

  6. Dynamics of electron solvation in methanol: Excited state relaxation and generation by charge-transfer-to-solvent

    SciTech Connect

    Elkins, Madeline H.; Williams, Holly L.; Neumark, Daniel M.

    2015-06-21

    The charge-transfer-to-solvent dynamics (CTTS) and excited state relaxation mechanism of the solvated electron in methanol are studied by time-resolved photoelectron spectroscopy on a liquid methanol microjet by means of two-pulse and three-pulse experiments. In the two-pulse experiment, CTTS excitation is followed by a probe photoejection pulse. The resulting time-evolving photoelectron spectrum reveals multiple time scales characteristic of relaxation and geminate recombination of the initially generated electron which are consistent with prior results from transient absorption. In the three-pulse experiment, the relaxation dynamics of the solvated electron following electronic excitation are measured. The internal conversion lifetime of the excited electron is found to be 130 ± 40 fs, in agreement with extrapolated results from clusters and the non-adiabatic relaxation mechanism.

  7. Charge transfer reactions in nematic liquid crystals

    SciTech Connect

    Wiederrecht, G.P.; Wasielewski, M.R. |; Galili, T.; Levanon, H.

    1998-07-01

    Ultrafast transient absorption studies of intramolecular photoinduced charge separation and thermal charge recombination were carried out on a molecule consisting of a 4-(N-pyrrolidino)naphthalene-1,8-imide donor (PNI) covalently attached to a pyromellitimide acceptor (PI) dissolved in the liquid crystal 4{prime}-(n-pentyl)-4-cyanobiphenyl (5CB). The temperature dependencies of the charge separation and recombination rates were obtained at temperatures above the nematic-isotropic phase transition of 5CB, where ordered microdomains exist and scattering of visible light by these domains is absent. The authors show that excited state charge separation is dominated by molecular reorientation of 5CB perpendicular to the director within the liquid crystal microdomains. They also show that charge recombination is adiabatic and is controlled by the comparatively slow collective reorientation of the liquid crystal microdomains relative to the orientation of PNI{sup +}-PI{sup {minus}}. They also report the results of time resolved electron paramagnetic resonance (TREPR) studies of photoinduced charge separation in a series of supramolecular compounds dissolved in oriented liquid crystal solvents. These studies permit the determination of the radical pair energy levels as the solvent reorganization energy increases from the low temperature crystalline phase, through the soft glass phase, to the nematic phase of the liquid crystal.

  8. Semiconductor nanorod liquid crystals

    SciTech Connect

    Li, Liang-shi; Walda, Joost; Manna, Liberato; Alivisatos, A. Paul

    2002-01-28

    Rodlike molecules form liquid crystalline phases with orientational order and positional disorder. The great majority of materials in which liquid crystalline phases have been observed are comprised of organic molecules or polymers, even though there has been continuing and growing interest in inorganic liquid crystals. Recent advances in the control of the sizes and shapes of inorganic nanocrystals allow for the formation of a broad class of new inorganic liquid crystals. Here we show the formation of liquid crystalline phases of CdSe semiconductor nanorods. These new liquid crystalline phases may have great importance for both application and fundamental study.

  9. Liquid level detector

    DOEpatents

    Grasso, A.P.

    1984-02-21

    A liquid level detector for low pressure boilers. A boiler tank, from which vapor, such as steam, normally exits via a main vent, is provided with a vertical side tube connected to the tank at the desired low liquid level. When the liquid level falls to the level of the side tube vapor escapes therethrough causing heating of a temperature sensitive device located in the side tube, which, for example, may activate a liquid supply means for adding liquid to the boiler tank. High liquid level in the boiler tank blocks entry of vapor into the side tube, allowing the temperature sensitive device to cool, for example, to ambient temperature.

  10. Liquid level detector

    DOEpatents

    Grasso, Albert P.

    1986-01-01

    A liquid level detector for low pressure boilers. A boiler tank, from which apor, such as steam, normally exits via a main vent, is provided with a vertical side tube connected to the tank at the desired low liquid level. When the liquid level falls to the level of the side tube vapor escapes therethrough causing heating of a temperature sensitive device located in the side tube, which, for example, may activate a liquid supply means for adding liquid to the boiler tank. High liquid level in the boiler tank blocks entry of vapor into the side tube, allowing the temperature sensitive device to cool, for example, to ambient temperature.

  11. Atmospheric Excitation of Planetary Normal Modes

    NASA Technical Reports Server (NTRS)

    Tanimoto, Toshiro

    2001-01-01

    The objectives of this study were to: (1) understand the phenomenon of continuous free oscillations of the Earth and (2) examine the idea of using this phenomenon for planetary seismology. We first describe the results on (1) and present our evaluations of the idea (2) in the final section. In 1997, after almost forty years since the initial attempt by Benioff et al, continuous free oscillations of the Earth were discovered. Spheroidal fundamental modes between 2 and 7 millihertz are excited continuously with acceleration amplitudes of about 0.3-0.5 nanogals. The signal is now commonly found in virtually all data recorded by STS-1 type broadband seismometers at quiet sites. Seasonal variation in amplitude and the existence of two coupled modes between the atmosphere and the solid Earth support that these oscillations are excited by the atmosphere. Stochastic excitation due to atmospheric turbulence is a favored mechanism, providing a good match between theory and data. The atmosphere has ample energy to support this theory because excitation of these modes require only 500-10000 W whereas the atmosphere contains about 117 W of kinetic energy. An application of this phenomenon includes planetary seismology, because other planets may be oscillating due to atmospheric excitation. The interior structure of planets could be learned by determining the eigenfrequencies in the continuous free oscillations. It is especially attractive to pursue this idea for tectonically quiet planets, since quakes may be too infrequent to be recorded by seismic instruments.

  12. Tone-excited jet: Theory and experiments

    NASA Technical Reports Server (NTRS)

    Ahuja, K. K.; Lepicovsky, J.; Tam, C. K. W.; Morris, P. J.; Burrin, R. H.

    1982-01-01

    A detailed study to understand the phenomenon of broadband jet-noise amplification produced by upstream discrete-tone sound excitation has been carried out. This has been achieved by simultaneous acquisition of the acoustic, mean velocity, turbulence intensities, and instability-wave pressure data. A 5.08 cm diameter jet has been tested for this purpose under static and also flight-simulation conditions. An open-jet wind tunnel has been used to simulate the flight effects. Limited data on heated jets have also been obtained. To improve the physical understanding of the flow modifications brought about by the upstream discrete-tone excitation, ensemble-averaged schlieren photographs of the jets have also been taken. Parallel to the experimental study, a mathematical model of the processes that lead to broadband-noise amplification by upstream tones has been developed. Excitation of large-scale turbulence by upstream tones is first calculated. A model to predict the changes in small-scale turbulence is then developed. By numerically integrating the resultant set of equations, the enhanced small-scale turbulence distribution in a jet under various excitation conditions is obtained. The resulting changes in small-scale turbulence have been attributed to broadband amplification of jet noise. Excellent agreement has been found between the theory and the experiments. It has also shown that the relative velocity effects are the same for the excited and the unexcited jets.

  13. "Safe" Coulomb excitation of 30Mg.

    PubMed

    Niedermaier, O; Scheit, H; Bildstein, V; Boie, H; Fitting, J; von Hahn, R; Köck, F; Lauer, M; Pal, U K; Podlech, H; Repnow, R; Schwalm, D; Alvarez, C; Ames, F; Bollen, G; Emhofer, S; Habs, D; Kester, O; Lutter, R; Rudolph, K; Pasini, M; Thirolf, P G; Wolf, B H; Eberth, J; Gersch, G; Hess, H; Reiter, P; Thelen, O; Warr, N; Weisshaar, D; Aksouh, F; Van den Bergh, P; Van Duppen, P; Huyse, M; Ivanov, O; Mayet, P; Van de Walle, J; Aystö, J; Butler, P A; Cederkäll, J; Delahaye, P; Fynbo, H O U; Fraile, L M; Forstner, O; Franchoo, S; Köster, U; Nilsson, T; Oinonen, M; Sieber, T; Wenander, F; Pantea, M; Richter, A; Schrieder, G; Simon, H; Behrens, T; Gernhäuser, R; Kröll, T; Krücken, R; Münch, M; Davinson, T; Gerl, J; Huber, G; Hurst, A; Iwanicki, J; Jonson, B; Lieb, P; Liljeby, L; Schempp, A; Scherillo, A; Schmidt, P; Walter, G

    2005-05-01

    We report on the first radioactive beam experiment performed at the recently commissioned REX-ISOLDE facility at CERN in conjunction with the highly efficient gamma spectrometer MINIBALL. Using 30Mg ions accelerated to an energy of 2.25 MeV/u together with a thin (nat)Ni target, Coulomb excitation of the first excited 2+ states of the projectile and target nuclei well below the Coulomb barrier was observed. From the measured relative deexcitation gamma-ray yields the B(E2;0(+)gs-->2(+)1) value of 30Mg was determined to be 241(31)e2 fm4. Our result is lower than values obtained at projectile fragmentation facilities using the intermediate-energy Coulomb excitation method, and confirms the theoretical conjecture that the neutron-rich magnesium isotope 30Mg resides outside the "island of inversion."

  14. Bernoulli excitation and detection of gas bubbles.

    PubMed

    Telling, R H; Walton, A J

    2001-10-01

    A simple method is proposed for detecting and sizing bubbles in pipeline fluid flow. This is based on changing the pressure of the fluid, which in turn excites volume oscillations in the bubble. If the change in pressure is of sufficient brevity and magnitude, the transient distortion results in excitation of the bubble into radiative oscillation at its natural frequency. In a moving fluid, the Bernoulli equation predicts that such a pressure change can be achieved through a suitable gradient in the flow velocity. In the experiments described here, this is achieved by altering the cross-sectional area of the pipe in which the fluid is flowing. We demonstrate the efficacy of this excitation method and, by detecting the radiated sound using a nearby hydrophone, determine the size of individual bubbles from their characteristic oscillation frequency.

  15. Charge-displacement analysis for excited states

    SciTech Connect

    Ronca, Enrico Tarantelli, Francesco; Pastore, Mariachiara Belpassi, Leonardo; De Angelis, Filippo; Angeli, Celestino; Cimiraglia, Renzo

    2014-02-07

    We extend the Charge-Displacement (CD) analysis, already successfully employed to describe the nature of intermolecular interactions [L. Belpassi et al., J. Am. Chem. Soc. 132, 13046 (2010)] and various types of controversial chemical bonds [L. Belpassi et al., J. Am. Chem. Soc. 130, 1048 (2008); N. Salvi et al., Chem. Eur. J. 16, 7231 (2010)], to study the charge fluxes accompanying electron excitations, and in particular the all-important charge-transfer (CT) phenomena. We demonstrate the usefulness of the new approach through applications to exemplary excitations in a series of molecules, encompassing various typical situations from valence, to Rydberg, to CT excitations. The CD functions defined along various spatial directions provide a detailed and insightful quantitative picture of the electron displacements taking place.

  16. Charge-displacement analysis for excited states

    NASA Astrophysics Data System (ADS)

    Ronca, Enrico; Pastore, Mariachiara; Belpassi, Leonardo; De Angelis, Filippo; Angeli, Celestino; Cimiraglia, Renzo; Tarantelli, Francesco

    2014-02-01

    We extend the Charge-Displacement (CD) analysis, already successfully employed to describe the nature of intermolecular interactions [L. Belpassi et al., J. Am. Chem. Soc. 132, 13046 (2010)] and various types of controversial chemical bonds [L. Belpassi et al., J. Am. Chem. Soc. 130, 1048 (2008); N. Salvi et al., Chem. Eur. J. 16, 7231 (2010)], to study the charge fluxes accompanying electron excitations, and in particular the all-important charge-transfer (CT) phenomena. We demonstrate the usefulness of the new approach through applications to exemplary excitations in a series of molecules, encompassing various typical situations from valence, to Rydberg, to CT excitations. The CD functions defined along various spatial directions provide a detailed and insightful quantitative picture of the electron displacements taking place.

  17. Asymptotic wave propagation in excitable media.

    PubMed

    Bernus, Olivier; Vigmond, Edward

    2015-07-01

    Wave shape and velocity are important issues in reaction-diffusion systems, and are often the result of competition in media with heterogeneous conduction properties. Asymptotic wave front propagation at maximal conduction velocity has been previously reported in the context of anisotropic cardiac tissue, but it is unknown whether this is a universal property of excitable tissues where conduction velocity can be locally modulated by mechanisms other than anisotropy. Here, we investigate the impact of conduction heterogeneities and boundary effects on wave propagation in excitable media. Following a theoretical analysis, we find that wave-front cusps occur where local velocity is reduced and that asymptotic wave fronts propagate at the maximal translational conduction velocity. Simulations performed in different reaction-diffusion systems, including cardiac tissue, confirm our theoretical findings. We conclude that this property can be found in a wide range of reaction-diffusion systems with excitable dynamics and that asymptotic wave-front shapes can be predicted.

  18. Shear layer excitation, experiment versus theory

    NASA Technical Reports Server (NTRS)

    Bechert, D. W.; Stahl, B.

    1984-01-01

    The acoustical excitation of shear layers is investigated. Acoustical excitation causes the so-called orderly structures in shear layers and jets. Also, the deviations in the spreading rate between different shear layer experiments are due to the same excitation mechanism. Measurements in the linear interaction region close to the edge from which the shear layer is shed are examined. Two sets of experiments (Houston 1981 and Berlin 1983/84) are discussed. The measurements were carried out with shear layers in air using hot wire anemometers and microphones. The agreement between these measurements and the theory is good. Even details of the fluctuating flow field correspond to theoretical predictions, such as the local occurrence of negative phase speeds.

  19. Artificial Excitation of Schumann Resonance with HAARP

    NASA Astrophysics Data System (ADS)

    Streltsov, A. V.; Chang, C. L.

    2014-12-01

    We report results from the experiment aimed at the artificial excitation of extremely-low-frequency (ELF) electromagnetic waves with frequencies corresponding to the frequency of Schumann resonance (typically, 7.5 - 8.0 Hz frequency range). Electromagnetic waves with these frequencies can form a standing pattern inside the spherical cavity formed by the surface of the earth and the ionosphere. In the experiment the ELF waves were excited by heating the ionosphere with X-mode HF electromagnetic waves generated by the High Frequency Active Auroral Research Program (HAARP) facility in Alaska. The experiment demonstrates that heating of the ionosphere can excite relatively large-amplitude electromagnetic waves with frequencies in the range of the Schumann resonance, when the ionosphere has a strong F-layer and an electric field greater than 5 mV/m is present in the E-region.

  20. Asymmetric Magnon Excitation by Spontaneous Toroidal Ordering

    NASA Astrophysics Data System (ADS)

    Hayami, Satoru; Kusunose, Hiroaki; Motome, Yukitoshi

    2016-05-01

    The effects of spontaneous toroidal ordering on magnetic excitation are theoretically investigated for a localized spin model that includes a staggered Dzyaloshinsky-Moriya interaction and anisotropic exchange interactions, which arise from the antisymmetric spin-orbit coupling and the multiorbital correlation effect. We show that the model exhibits a Néel-type antiferromagnetic order, which simultaneously accompanies a ferroic toroidal order. We find that the occurrence of toroidal order modulates the magnon dispersion in an asymmetric way with respect to the wave number: a toroidal dipole order on the zigzag chain leads to a band-bottom shift, while a toroidal octupole order on the honeycomb lattice gives rise to a valley splitting. These asymmetric magnon excitations could be a source of unusual magnetic responses, such as nonreciprocal magnon transport. A variety of modulations are discussed while changing the lattice and magnetic symmetries. The implications regarding candidate materials for asymmetric magnon excitations are presented.

  1. Excitation of gravity waves in common envelopes

    NASA Technical Reports Server (NTRS)

    Soker, Noam

    1992-01-01

    We study the excitation of gravity waves by a low-mass companion orbiting inside the envelope of a giant star, concentrating on brown dwarfs inside the envelope of asymptotic giant branch stars. Efficient g-wave excitations occur only after the brown dwarf has spiraled-in to the radiative zone, well inside the envelope, of the asymptotic giant branch star. The brown dwarf excites g-waves when its orbital radius is about 3-10 solar radii. At this stage of the evolution the envelope mass is below 0.1 solar mass. The g-waves propagate inward from the secondary orbit, carrying angular momentum and energy. We find that the angular momentum transport leads to an efficient spin-up of the inner envelopes. The differential rotation between the envelope and core and nonlinear wave effects, can cause a mixing of heavy elements from the core to the envelope.

  2. Nanoscale control of phonon excitations in graphene

    PubMed Central

    Kim, Hyo Won; Ko, Wonhee; Ku, JiYeon; Jeon, Insu; Kim, Donggyu; Kwon, Hyeokshin; Oh, Youngtek; Ryu, Seunghwa; Kuk, Young; Hwang, Sung Woo; Suh, Hwansoo

    2015-01-01

    Phonons, which are collective excitations in a lattice of atoms or molecules, play a major role in determining various physical properties of condensed matter, such as thermal and electrical conductivities. In particular, phonons in graphene interact strongly with electrons; however, unlike in usual metals, these interactions between phonons and massless Dirac fermions appear to mirror the rather complicated physics of those between light and relativistic electrons. Therefore, a fundamental understanding of the underlying physics through systematic studies of phonon interactions and excitations in graphene is crucial for realising graphene-based devices. In this study, we demonstrate that the local phonon properties of graphene can be controlled at the nanoscale by tuning the interaction strength between graphene and an underlying Pt substrate. Using scanning probe methods, we determine that the reduced interaction due to embedded Ar atoms facilitates electron–phonon excitations, further influencing phonon-assisted inelastic electron tunnelling. PMID:26109454

  3. Excitation spectrum of the attractive Hubbard model

    SciTech Connect

    Micnas, R.; Pedersen, M.H.; Schafroth, S.; Schneider, T.; Rodriguez-Nunez, J.J.; Beck, H.

    1995-12-01

    We study excitation-spectrum and normal-state properties of the two-dimensional attractive Hubbard model using the conserving, self-consistent {ital T}-matrix formalism in the intermediate coupling regime and at low electron concentration. Numerical results are presented for one-particle and two-particle excitation spectra, the one-particle momentum distribution, the chemical potential, and the static spin susceptibility. For a coupling strength of {ital U}/{ital t}=4.0, the one-particle spectral function, {ital A}(k,{omega}), shows two peaks of different weights. One peak can be associated with pair formation, whereas the other corresponds to renormalized quasiparticle excitation. It turns out that the two-band feature is reasonably well described by an ansatz for {ital A}(k,{omega}), which satisfies the first four frequency moments.

  4. Excited light meson spectroscopy from lattice QCD

    SciTech Connect

    Christopher Thomas, Hadron Spectrum Collaboration

    2012-04-01

    I report on recent progress in calculating excited meson spectra using lattice QCD, emphasizing results and phenomenology. With novel techniques we can now extract extensive spectra of excited mesons with high statistical precision, including spin-four states and those with exotic quantum numbers. As well as isovector meson spectra, I will present new calculations of the spectrum of excited light isoscalar mesons, something that has up to now been a challenge for lattice QCD. I show determinations of the flavor content of these mesons, including the eta-eta' mixing angle, providing a window on annihilation dynamics in QCD. I will also discuss recent work on using lattice QCD to map out the energy-dependent phase shift in pi-pi scattering and future applications of the methodology to the study of resonances and decays.

  5. Electron-impact vibrational excitation of cyclopropane

    SciTech Connect

    Čurík, R. Čársky, P.; Allan, M.

    2015-04-14

    We report a very detailed test of the ab initio discrete momentum representation (DMR) method of calculating vibrational excitation of polyatomic molecules by electron impact, by comparison of its results with an extensive set of experimental data, covering the entire range of scattering angles from 10{sup ∘} to 180{sup ∘} and electron energies from 0.4 to 20 eV. The DMR calculations were carried out by solving the two-channel Lippmann-Schwinger equation in the momentum space, and the interaction between the scattered electron and the target molecule was described by exact static-exchange potential corrected by a density functional theory (DFT) correlation-polarization interaction that models target’s response to the field of incoming electron. The theory is found to quantitatively reproduce the measured spectra for all normal modes, even at the difficult conditions of extreme angles and at low energies, and thus provides full understanding of the excitation mechanism. It is shown that the overlap of individual vibrational bands caused by limited experimental resolution and rotational excitation must be properly taken into account for correct comparison of experiment and theory. By doing so, an apparent discrepancy between published experimental data could be reconciled. A substantial cross section is found for excitation of the non-symmetric HCH twisting mode ν{sub 4} of A{sub 1}{sup ″} symmetry by the 5.5 eV A{sub 2}{sup ′} resonance, surprisingly because the currently accepted selection rules predict this process to be forbidden. The DMR theory shows that the excitation is caused by an incoming electron in an f-wave of A{sub 2}{sup ′} symmetry which causes excitation of the non-symmetric HCH twisting mode ν{sub 4} of the A{sub 1}{sup ″} symmetry and departs in p- and f-waves of A{sub 2}{sup ″} symmetry.

  6. Electron-impact vibrational excitation of cyclopropane.

    PubMed

    Čurík, R; Čársky, P; Allan, M

    2015-04-14

    We report a very detailed test of the ab initio discrete momentum representation (DMR) method of calculating vibrational excitation of polyatomic molecules by electron impact, by comparison of its results with an extensive set of experimental data, covering the entire range of scattering angles from 10° to 180° and electron energies from 0.4 to 20 eV. The DMR calculations were carried out by solving the two-channel Lippmann-Schwinger equation in the momentum space, and the interaction between the scattered electron and the target molecule was described by exact static-exchange potential corrected by a density functional theory (DFT) correlation-polarization interaction that models target's response to the field of incoming electron. The theory is found to quantitatively reproduce the measured spectra for all normal modes, even at the difficult conditions of extreme angles and at low energies, and thus provides full understanding of the excitation mechanism. It is shown that the overlap of individual vibrational bands caused by limited experimental resolution and rotational excitation must be properly taken into account for correct comparison of experiment and theory. By doing so, an apparent discrepancy between published experimental data could be reconciled. A substantial cross section is found for excitation of the non-symmetric HCH twisting mode ν4 of A1 (″) symmetry by the 5.5 eV A2 (') resonance, surprisingly because the currently accepted selection rules predict this process to be forbidden. The DMR theory shows that the excitation is caused by an incoming electron in an f-wave of A2 (') symmetry which causes excitation of the non-symmetric HCH twisting mode ν4 of the A1 (″) symmetry and departs in p- and f-waves of A2 (″) symmetry. PMID:25877583

  7. Precision liquid level sensor

    DOEpatents

    Field, M.E.; Sullivan, W.H.

    A precision liquid level sensor utilizes a balanced bridge, each arm including an air dielectric line. Changes in liquid level along one air dielectric line imbalance the bridge and create a voltage which is directly measurable across the bridge.

  8. Zero gravity liquid mixer

    NASA Technical Reports Server (NTRS)

    Booth, F. W.; Bruce, R. A. (Inventor)

    1973-01-01

    An apparatus for mixing liquids under conditions of zero gravity is disclosed. The apparatus is comprised of a closed reservoir for the liquids, with a means for maintaining a positive pressure on the liquids in the reservoir. A valved liquid supply line is connected to the reservoir for supplying the reservoir with the liquids to be mixed in the reservoir. The portion of the reservoir containing the liquids to be mixed is in communication with a pump which alternately causes a portion of the liquids to flow out of the pump and into the reservoir to mix the liquids. The fluids in the reservoir are in communication through a conduit with the pump which alternately causes a portion of the fluids to flow out of the pump and into the sphere. The conduit connecting the pump and sphere may contain a nozzle or other jet-forming structure such as a venturi for further mixing the fluids.

  9. Liquid medication administration

    MedlinePlus

    ... easily. Oral syringes have some advantages for giving liquid medicines. They are accurate. They are easy to ... cups are also a handy way to give liquid medicines. However, dosing errors have occurred with them. ...

  10. Optical Excitation and Probing of Bottle Microresonators

    NASA Astrophysics Data System (ADS)

    Murugan, G. Senthil; Wilkinson, J. S.; Zervas, M. N.

    2010-11-01

    Fiber bottle microresonators supporting helical whispering gallery modes and exhibiting field maxima symmetrically located on either side of the neck of the bottle have been demonstrated. Channel dropping characteristics have been studied experimentally for the first time in this type of microresonator, using tapered excitation and probe fibers symmetrically placed on both sides of the bottle microresonator. Selective excitation on one side of the bottle microresonator leads to symmetrically located turning points and power localization on both sides of the bottle, leading to the potential to construct add-drop filters.

  11. The resonance Raman excitation profile of fucoxanthin

    NASA Astrophysics Data System (ADS)

    Ballard, L. J.; Glasgow, L. A.; Hoskins, L. C.; Krohe, T.

    1989-01-01

    The resonance Raman excitation profiles (RREPs) of the ν 1 and ν 2 vibrations of fucoxanthin in acetone and toluene solvents have been studied. Fucoxanthin, which is a predominant pigment in marine seaweed and phytoplankton, has several structural differences from carotenoids for which excitation profiles have been determined. The RREPs for fucoxanthin are interpreted in terms of a two-mode model and show a B2 value which is approximately 20% lower than for carotenoids like β-carotene and lutein which occur in higher plants. Excellent fits between experimental data and the theoretical model were observed in both solvents.

  12. Charmonium excited state spectrum in lattice QCD

    SciTech Connect

    Jozef Dudek; Robert Edwards; Nilmani Mathur; David Richards

    2008-02-01

    Working with a large basis of covariant derivative-based meson interpolating fields we demonstrate the feasibility of reliably extracting multiple excited states using a variational method. The study is performed on quenched anisotropic lattices with clover quarks at the charm mass. We demonstrate how a knowledge of the continuum limit of a lattice interpolating field can give additional spin-assignment information, even at a single lattice spacing, via the overlap factors of interpolating field and state. Excited state masses are systematically high with respect to quark potential model predictions and, where they exist, experimental states. We conclude that this is most likely a result of the quenched approximation.

  13. Selective form of an excitable membrane plasticity.

    PubMed

    Tsitolovsky, L E; Babkina, N V

    1992-11-01

    This work describes the change in an active electrogenesis of the command neurons responsible for defensive closure of a snail's pneumostome during elaborating, extinction and restoration of a classical conditioned defensive reflex to a tactile stimulus. Tactile stimulations applied to different parts of a snail's body served as a differential stimulus. As the biological value of a conditioned stimulus increases due to learning, the excitability of command neurons in response to conditioned stimulus rises. At the same time the neurons demonstrated a reduced excitability in response to a differentiating stimulus.

  14. Wave instabilities in an excitable electrochemical system

    NASA Astrophysics Data System (ADS)

    Otterstedt, R. D.; Jaeger, N. I.; Plath, P. J.; Hudson, J. L.

    1998-11-01

    Spatiotemporal pattern formation under potentiostatic control in the excitable potential range at the active/passive transition of cobalt in buffered phosphoric acid has been investigated in a ribbon electrode geometry. The propagation of an active area with modulation and wave splitting has been observed, depending on the parameters potential and time of passivation prior to excitation. The modulation and wave splitting are influenced both by the kinetics of repassivation on the electrode surface and by long-range coupling and positive feedback through the electric field. Modulation in the vicinity of the system boundary gives rise to an apparent reflection of the active area at the boundary.

  15. Collective charge excitations along cell membranes

    NASA Astrophysics Data System (ADS)

    Manousakis, E.

    2005-07-01

    A significant part of the thin layers of counter-ions adjacent to the exterior and interior surfaces of a cell membrane form quasi-two-dimensional (2D) layers of mobile charge. Collective charge density oscillations, known as plasmon modes, in these 2D charged systems of counter-ions are predicted in the present paper. This is based on a calculation of the self-consistent response of this system to a fast electric field fluctuation. The possibility that the membrane channels might be using these excitations to carry out fast communication is suggested and experiments are proposed to reveal the existence of such excitations.

  16. Exciting Baryons: now and in the future

    SciTech Connect

    Michael Pennington

    2012-04-01

    This is the final talk of NSTAR2011 conference. It is not a summary talk, but rather a looking forward to what still needs to be done in excited baryon physics. In particular, we need to hone our tools connecting experimental inputs with QCD. At present we rely on models that often have doubtful connections with the underlying theory, and this needs to be dramatically improved, if we are to reach definitive conclusions about the relevant degrees of freedom of excited baryons. Conclusions that we want to have by NSTAR2021.

  17. Exciting baryons: Now and in the future

    NASA Astrophysics Data System (ADS)

    Pennington, M. R.

    2012-04-01

    This is the final talk of NSTAR2011 conference. It is not a summary talk, but rather a looking forward to what still needs to be done in excited baryon physics. In particular, we need to hone our tools connecting experimental inputs with QCD. At present we rely on models that often have doubtful connections with the underlying theory, and this needs to be dramatically improved, if we are to reach definitive conclusions about the relevant degrees of freedom of excited baryons. Conclusions that we want to have by NSTAR2021.

  18. Double Photoionization of excited Lithium and Beryllium

    SciTech Connect

    Yip, Frank L.; McCurdy, C. William; Rescigno, Thomas N.

    2010-05-20

    We present total, energy-sharing and triple differential cross sections for one-photon, double ionization of lithium and beryllium starting from aligned, excited P states. We employ a recently developed hybrid atomic orbital/ numerical grid method based on the finite-element discrete-variable representation and exterior complex scaling. Comparisons with calculated results for the ground-state atoms, as well as analogous results for ground-state and excited helium, serve to highlight important selection rules and show some interesting effects that relate to differences between inter- and intra-shell electron correlation.

  19. Elementary spin excitations in ultrathin itinerant magnets

    NASA Astrophysics Data System (ADS)

    Zakeri, Khalil

    2014-12-01

    Elementary spin excitations (magnons) play a fundamental role in condensed matter physics, since many phenomena e.g. magnetic ordering, electrical (as well as heat) transport properties, ultrafast magnetization processes, and most importantly electron/spin dynamics can only be understood when these quasi-particles are taken into consideration. In addition to their fundamental importance, magnons may also be used for information processing in modern spintronics. Here the concept of spin excitations in ultrathin itinerant magnets is discussed and reviewed. Starting with a historical introduction, different classes of magnons are introduced. Different theoretical treatments of spin excitations in solids are outlined. Interaction of spin-polarized electrons with a magnetic surface is discussed. It is shown that, based on the quantum mechanical conservation rules, a magnon can only be excited when a minority electron is injected into the system. While the magnon creation process is forbidden by majority electrons, the magnon annihilation process is allowed instead. These fundamental quantum mechanical selection rules, together with the strong interaction of electrons with matter, make the spin-polarized electron spectroscopies as appropriate tools to excite and probe the elementary spin excitations in low-dimensional magnets e.g ultrathin films and nanostructures. The focus is put on the experimental results obtained by spin-polarized electron energy loss spectroscopy and spin-polarized inelastic tunneling spectroscopy. The magnon dispersion relation, lifetime, group and phase velocity measured using these approaches in various ultrathin magnets are discussed in detail. The differences and similarities with respect to the bulk excitations are addressed. The role of the temperature, atomic structure, number of atomic layers, lattice strain, electronic complexes and hybridization at the interfaces are outlined. A possibility of simultaneous probing of magnons and phonons

  20. Laser Excited Fluorescence For Forensic Diagnostics

    NASA Astrophysics Data System (ADS)

    McKinney, Robert E.

    1986-07-01

    The application of laser excited fluorescence to the detection and identification of latent fingerprints was first accomplished ten years ago. The development of the technology has progressed rapidly with the introduction of commercial equipment by several manufacturers. Systems based on Argon-ion, Copper-vapor, and frequency-doubled Nd:YAG lasers are compared. The theoretical basis of detection by fluorescence is discussed along with the more useful techniques of dye staining. Other applications of the laser excited fluorescence in forensic investigation include gunshot residue analysis, serology, collection of trace evidence, and document examination.

  1. Optimal Parametric Feedback Excitation of Nonlinear Oscillators

    NASA Astrophysics Data System (ADS)

    Braun, David J.

    2016-01-01

    An optimal parametric feedback excitation principle is sought, found, and investigated. The principle is shown to provide an adaptive resonance condition that enables unprecedentedly robust movement generation in a large class of oscillatory dynamical systems. Experimental demonstration of the theory is provided by a nonlinear electronic circuit that realizes self-adaptive parametric excitation without model information, signal processing, and control computation. The observed behavior dramatically differs from the one achievable using classical parametric modulation, which is fundamentally limited by uncertainties in model information and nonlinear effects inevitably present in real world applications.

  2. Optimal Parametric Feedback Excitation of Nonlinear Oscillators.

    PubMed

    Braun, David J

    2016-01-29

    An optimal parametric feedback excitation principle is sought, found, and investigated. The principle is shown to provide an adaptive resonance condition that enables unprecedentedly robust movement generation in a large class of oscillatory dynamical systems. Experimental demonstration of the theory is provided by a nonlinear electronic circuit that realizes self-adaptive parametric excitation without model information, signal processing, and control computation. The observed behavior dramatically differs from the one achievable using classical parametric modulation, which is fundamentally limited by uncertainties in model information and nonlinear effects inevitably present in real world applications. PMID:26871336

  3. Liquid level sensing device

    DOEpatents

    Tokarz, Richard D.

    1983-01-01

    A liquid level sensing device comprising a load cell supporting a column or stack of segments freely resting on one another. The density of each element is substantially identical to that of the surrounding liquid. The elements are freely guided within a surrounding tube. As each element is exposed above the liquid level, its weight will be impressed through the column to the load cell, thereby providing a signal at the load cell directly proportional to the liquid level elevation.

  4. Band excitation method applicable to scanning probe microscopy

    DOEpatents

    Jesse, Stephen; Kalinin, Sergei V.

    2015-08-04

    Scanning probe microscopy may include a method for generating a band excitation (BE) signal and simultaneously exciting a probe at a plurality of frequencies within a predetermined frequency band based on the excitation signal. A response of the probe is measured across a subset of frequencies of the predetermined frequency band and the excitation signal is adjusted based on the measured response.

  5. Fluid Mechanics of Liquid-Liquid Systems.

    NASA Astrophysics Data System (ADS)

    Richards, John Reed

    The detailed hydrodynamics of selected liquid -liquid flow systems are investigated to provide a firm foundation for the rational design of separation processes. The implementation of this objective centers on the development of a robust code to simulate liquid-liquid flows. We have applied this code to the realistic simulation of aspects of the complex fluid mechanical behavior, and developed quantitative insight into the underlying processes involved. The Volume of Fluid (VOF) method is combined with the Continuous Surface Force (CSF) algorithm to provide a numerically stable code capable of solving high Reynolds numbers free surface flows. One of the developments during the testing was an efficient method for solving the Young-Laplace equation describing the shape of the meniscus in a vertical cylinder for a constrained liquid volume. The steady-state region near the nozzle for the laminar flow of a Newtonian liquid jet injected vertically into another immiscible Newtonian liquid is investigated for various Reynolds numbers by solving the axisymmetric transient equations of motion and continuity. The analysis takes into account pressure, viscous, inertial, gravitational, and surface tension forces, and comparison with previous experimental measurements shows good agreement. Comparisons of the present numerical method with the numerical results of previous boundary-layer methods help establish their range of validity. A new approximate equation for the shape of the interface of the steady jet, based on an overall momentum balance, is also developed. The full transient from liquid-liquid jet startup to breakup into drops is also simulated numerically. In comparison with experiment, the results of the present numerical method show a greater sensitivity of the jet length to the Reynolds number than the best predictions of previous linear stability analyses. The formation of drops is investigated at low to high Reynolds numbers before and after jet formation. The

  6. Liquid detection circuit

    DOEpatents

    Regan, Thomas O.

    1987-01-01

    Herein is a circuit which is capable of detecting the presence of liquids, especially cryogenic liquids, and whose sensor will not overheat in a vacuum. The circuit parameters, however, can be adjusted to work with any liquid over a wide range of temperatures.

  7. Renewable liquid reflection grating

    DOEpatents

    Ryutov, Dmitri D.; Toor, Arthur

    2003-10-07

    A renewable liquid reflection grating. Electrodes are operatively connected to a conducting liquid in an arrangement that produces a reflection grating and driven by a current with a resonance frequency. In another embodiment, the electrodes create the grating by a resonant electrostatic force acting on a dielectric liquid.

  8. Liquid metal cold trap

    DOEpatents

    Hundal, Rolv

    1976-01-01

    A cold trap assembly for removing impurities from a liquid metal being provided with a hole between the incoming impure liquid metal and purified outgoing liquid metal which acts as a continuous bleed means and thus prevents the accumulation of cover gases within the cold trap assembly.

  9. PREFACE: 6th Liquid Matter Conference

    NASA Astrophysics Data System (ADS)

    Dijkstra, Marjolein; van Roij, René; Vroege, Gert Jan; Lekkerkerker, Henk; Frenkel, Daan

    2005-11-01

    This special issue of Journal of Physics: Condensed Matter contains the Proceedings of the 6th Liquid Matter Conference held in Utrecht, The Netherlands, 2-6 July 2005. The three-yearly Liquid Matter Conference is organized by the Liquids Section of the Condensed Matter Division of the European Physical Society. This series of meetings began in Lyon in 1990. The most recent meeting was held in 2003 in Konstanz. The aim of the Liquid Matter Conferences is to bring together scientists working on the liquid state of matter. This rapidly growing field includes the physics, chemistry, biology and chemical engineering of liquid matter as well as various applied research areas. In fact, the Utrecht meeting had, for the first time, a special session devoted to Fundamental Challenges in Applied Liquid Physics and Microfluidics. The Utrecht meeting had 760 registered participants from four continents. An important event at this meeting was the award of the First Liquid Matter Prize of the European Physical Society to Professor Jean-Pierre Hansen FRS, of Cambridge University. In addition to a plenary speech by the recipient of the Liquid Matter Prize, the scientific programme consisted of 10 plenary lectures, 117 symposia talks, 25 of which were keynote lectures and some 650 poster contributions. The meeting also hosted a one-day symposium of the Division of Liquids and Interfaces of the Chemical Sciences division of NWO. This special issue of Journal of Physics: Condensed Matter contains 61 of the oral communications. Liquid state physics is at the interface of many fields of research. As a consequence, many of the attendants come from adjacent fields and find in the Liquid Matter Conference a forum to meet experts from other areas of research. This aspect of the Liquid Matter Conference makes it an exciting meeting as it not only offers the participants an up-to-date picture of the status of research into the liquid state of matter, but it also allows them to establish new

  10. Room Temperature Single-Photon Source: Single-Dye Molecule Fluorescence in Liquid Crystal Host

    SciTech Connect

    Lukishova, S.G.; Schmid, A.W.; McNamara, A.J.; Boyd, R.W.; Stroud, C.R.Jr.

    2003-12-31

    OAK-(B204)We report on new approaches toward an implementation of an efficient, room temperature, deterministically polarized, single-photon source (SPS) on demand-a key hardware element for quantum information and quantum communication. Operation of a room temperature SPS is demonstrated via photon antibunching in the fluorescence from single terrylene-dye molecules embedded in a cholesteric liquid crystal host. Using oxygen-depleted liquid crystal hosts, dye-bleaching was avoided over the course of more than 1 h of continuous 532-nm excitation. Liquid crystal hosts (including liquid crystal oligomers/polymers) permit further increase of the efficiency of the source: (1) by aligning the dye molecules along a direction preferable for the maximum excitation efficiency; (2) by tuning a one-dimensional (1-D) photonic-band-gap microcavity of planar-aligned cholesteric (chiral nematic) liquid crystal layer to the dye fluorescence band.

  11. Comparison of vapor formation of water at the solid/water interface to colloidal solutions using optically excited gold nanostructures.

    PubMed

    Baral, Susil; Green, Andrew J; Livshits, Maksim Y; Govorov, Alexander O; Richardson, Hugh H

    2014-02-25

    The phase transformation properties of liquid water to vapor is characterized by optical excitation of the lithographically fabricated single gold nanowrenches and contrasted to the phase transformation properties of gold nanoparticles located and optically excited in a bulk solution system [two and three dimensions]. The 532 nm continuous wave excitation of a single gold nanowrench results in superheating of the water to the spinodal decomposition temperature of 580 ± 20 K with bubble formation below the spinodal decomposition temperature being a rare event. Between the spinodal decomposition temperature and the boiling point liquid water is trapped into a metastable state because a barrier to vapor nucleation exists that must be overcome before the thermodynamically stable state is realized. The phase transformation for an optically heated single gold nanowrench is different from the phase transformation of optically excited colloidal gold nanoparticles solution where collective heating effects dominates and leads to the boiling of the solution exactly at the boiling point. In the solution case, the optically excited ensemble of nanoparticles collectively raises the ambient temperature of water to the boiling point where liquid is converted into vapor. The striking difference in the boiling properties of the single gold nanowrench and the nanoparticle solution system can be explained in terms of the vapor-nucleation mechanism, the volume of the overheated liquid, and the collective heating effect. The interpretation of the observed regimes of heating and vaporization is consistent with our theoretical modeling. In particular, we explain with our theory why the boiling with the collective heating in a solution requires 3 orders of magnitude less intensity compared to the case of optically driven single nanowrench.

  12. Relaxation channels of multi-photon excited xenon clusters

    SciTech Connect

    Serdobintsev, P. Yu.; Melnikov, A. S.; Rakcheeva, L. P. Murashov, S. V.; Khodorkovskii, M. A.; Lyubchik, S.; Timofeev, N. A.; Pastor, A. A.

    2015-09-21

    The relaxation processes of the xenon clusters subjected to multi-photon excitation by laser radiation with quantum energies significantly lower than the thresholds of excitation of atoms and ionization of clusters were studied. Results obtained by means of the photoelectron spectroscopy method showed that desorption processes of excited atoms play a significant role in the decay of two-photon excited xenon clusters. A number of excited states of xenon atoms formed during this process were discovered and identified.

  13. Visible fiber lasers excited by GaN laser diodes

    NASA Astrophysics Data System (ADS)

    Fujimoto, Yasushi; Nakanishi, Jun; Yamada, Tsuyoshi; Ishii, Osamu; Yamazaki, Masaaki

    2013-07-01

    This paper describes and discusses visible fiber lasers that are excited by GaN laser diodes. One of the attractive points of visible light is that the human eye is sensitive to it between 400 and 700 nm, and therefore we can see applications in display technology. Of course, many other applications exist. First, we briefly review previously developed visible lasers in the gas, liquid, and solid-state phases and describe the history of primary solid-state visible laser research by focusing on rare-earth doped fluoride media, including glasses and crystals, to clarify the differences and the merits of primary solid-state visible lasers. We also demonstrate over 1 W operation of a Pr:WPFG fiber laser due to high-power GaN laser diodes and low-loss optical fibers (0.1 dB/m) made by waterproof fluoride glasses. This new optical fiber glass is based on an AlF3 system fluoride glass, and its waterproof property is much better than the well known fluoride glass of ZBLAN. The configuration of primary visible fiber lasers promises highly efficient, cost-effective, and simple laser systems and will realize visible lasers with photon beam quality and quantity, such as high-power CW or tunable laser systems, compact ultraviolet lasers, and low-cost ultra-short pulse laser systems. We believe that primary visible fiber lasers, especially those excited by GaN laser diodes, will be effective tools for creating the next generation of research and light sources.

  14. Multipurpose exciter with low phase noise

    NASA Technical Reports Server (NTRS)

    Conroy, B.; Le, D.

    1989-01-01

    Results of an effort to develop a lower-cost exciter with high stability, low phase noise, and controllable phase and frequency for use in Deep Space Network and Goldstone Solar System Radar applications are discussed. Included is a discussion of the basic concept, test results, plans, and concerns.

  15. 46 CFR 111.12-3 - Excitation.

    Code of Federal Regulations, 2010 CFR

    2010-10-01

    ... generator unless it is provided with a permanent magnet or a residual-magnetism-type exciter that has the... GUARD, DEPARTMENT OF HOMELAND SECURITY (CONTINUED) ELECTRICAL ENGINEERING ELECTRIC SYSTEMS-GENERAL... (incorporated by reference; see 46 CFR 110.10-1), except that those for mobile offshore drilling units must...

  16. 46 CFR 111.12-3 - Excitation.

    Code of Federal Regulations, 2011 CFR

    2011-10-01

    ... generator unless it is provided with a permanent magnet or a residual-magnetism-type exciter that has the... GUARD, DEPARTMENT OF HOMELAND SECURITY (CONTINUED) ELECTRICAL ENGINEERING ELECTRIC SYSTEMS-GENERAL... (incorporated by reference; see 46 CFR 110.10-1), except that those for mobile offshore drilling units must...

  17. Contemporary continuum QCD approaches to excited hadrons

    NASA Astrophysics Data System (ADS)

    El-Bennich, Bruno; Rojas, Eduardo

    2016-03-01

    Amongst the bound states produced by the strong interaction, radially excited meson and nucleon states offer an important phenomenological window into the long-range behavior of the coupling constant in Quantum Chromodynamics. We here report on some technical details related to the computation of the bound state's eigenvalue spectrum in the framework of Bethe-Salpeter and Faddeev equations.

  18. Supersolitons: Solitonic Excitations in Atomic Soliton Chains

    SciTech Connect

    Novoa, David; Michinel, Humberto; Perez-Garcia, Victor M.

    2008-10-03

    We show that, by tuning interactions in nonintegrable vector nonlinear Schroedinger equations modeling Bose-Einstein condensates and other relevant physical systems, it is possible to achieve a regime of elastic particlelike collisions between solitons. This would allow one to construct a Newton's cradle with solitons and supersolitons: localized collective excitations in solitary-wave chains.

  19. Ionic electrostatic excitations along biological membranes

    NASA Astrophysics Data System (ADS)

    Moradi, Afshin

    2011-02-01

    A theoretical analysis of ionic electrostatic excitations of a charged biological membrane is presented within the framework of the fluid theory for surface ions inside and outside the cell, in conjunction with the Poisson's equation. General expressions of dispersion relations are obtained for electrostatic oscillations of intrinsic cellular with different shapes and symmetries.

  20. Excitation system for rotating synchronous machines

    DOEpatents

    Umans, Stephen D.; Driscoll, David J.

    2002-01-01

    A system for providing DC current to a rotating superconducting winding is provided. The system receives current feedback from the superconducting winding and determines an error signal based on the current feedback and a reference signal. The system determines a control signal corresponding to the error signal and provides a positive and negative superconducting winding excitation voltage based on the control signal.