Sequential character of low-energy ternary and quaternary nuclear fission

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kadmensky, S. G., E-mail: kadmensky@phys.vsu.ru; Bulychev, A. O.

2016-09-15

An analysis of low-energy true ternary (quaternary) nuclear fission leads to the conclusion that these fission modes have a sequential two-step (three-step) character such that the emission of a third particle (third and fourth particles) and the separation of fission fragments occur at distinctly different instants, in contrast to the simultaneous emergence of all fission products in the case of onestep ternary (quaternary) fission. This conclusion relies on the following arguments. First, the emission of a third particle (third and fourth particles) from a fissile nucleus is due to a nonevaporative mechanism associated with a nonadiabatic character of the collectivemore » deformation motion of this nucleus at the stages preceding its scission. Second, the axial symmetry of the deformed fissile compound nucleus and the direction of its symmetry axis both remain unchanged at all stages of ternary (quaternary) fission. This circumstancemakes it possible to explain themechanism of the appearance of observed anisotropies and T — odd asymmeries in the angular distributions of products of ternary (quaternary) nuclear fission. Third, the T —odd asymmetry discovered experimentally in ternary nuclear fission induced by cold polarized neutrons obeys the T —invariance condition only in the case of a sequential two-step (three-step) character of true ternary (quaternary) nuclear fission. At the same time, this asymmetry is not a T —invariant quantity in the case of the simultaneous emission of products of true ternary (quaternary) nuclear fission from the fissile compound nucleus.« less

Interference of fission amplitudes of neutron resonances and T-odd asymmetry for various prescission third particles in the ternary fission of nuclei

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kadmensky, S. G., E-mail: kadmensky@phys.vsu.ru; Bunakov, V. E.; Kadmensky, S. S.

Differential cross sections for reactions of the true ternary fission of nuclei that was induced by cold polarized neutrons were constructed with allowance of the effect that Coriolis interaction and the interference between fission amplitudes of neutron resonances excited in fissile nuclei upon incidentneutron capture by target nuclei exerted on angular distributions of prescission third particles (alpha particles, neutrons, or photons). It is shown that T -odd TRI- and ROT-type asymmetries for prescission alpha particles are associated with, respectively, the odd and even components of the Coriolis interaction-perturbed amplitude of angular distributions of particles belonging to the types indicated above.more » These asymmetries have angular distributions differing from each other and stemming from a nontrivial dependence of these components on the neutron-resonance spins J{sub s} and their projections K{sub s} onto the symmetry axis of the nucleus involved. It is shown that angular distributions of prescission photons and neutrons from reactions of the ternary fission of nuclei that is induced by cold polarized neutrons are determined by the effect of Coriolis forces exclusively. Therefore, the emerging T-odd asymmetries have a character of a ROT-type asymmetry and are universal for all target nuclei.« less

Low-spin structure of 51,35,86Br and 50,36,86Kr nuclei: The role of the g7 /2 neutron orbital

NASA Astrophysics Data System (ADS)

Urban, W.; Sieja, K.; Materna, T.; Czerwiński, M.; Rząca-Urban, T.; Blanc, A.; Jentschel, M.; Mutti, P.; Köster, U.; Soldner, T.; de France, G.; Simpson, G. S.; Ur, C. A.; Bernards, C.; Fransen, C.; Jolie, J.; Regis, J.-M.; Thomas, T.; Warr, N.

2016-10-01

Low-spin excited levels in 51,35,86Br and 50,36,86Kr, populated following β- decay and the neutron-induced fission of 235U, were measured using the Lohengrin fission-fragment separator and the EXILL array of Ge detectors at the PF1B cold-neutron facility of the Institute Laue-Langevin Grenoble. Improved populations of excited levels in 86Br remove inconsistencies existing in the literature on this nucleus. Directional-linear-polarization correlations, analyzed using newly developed formulas, as well as precise angular correlations allowed the unique 1- and 2- spin and parity assignments to the ground state of 86Br and the 4016.3-keV level in 86Kr, respectively. Based on these results we propose that the Gamow-Teller β- decays of 86Se and 86Br involve the ν g7 /2→π g9 /2 transition in addition to the ν p3 /2→π p3 /2 transition proposed earlier. In 86Kr we have identified 11+, 23+, and 31+ levels, analogous to the mixed-symmetry states in 94Mo, which in 86Kr are from proton excitations, only. Large-scale, shell-model calculations with refined interactions reproduce well excitations in 86Br and 86Kr and support our interpretations.

Survival Mediated Heavy Element Capture Cross Sections

NASA Astrophysics Data System (ADS)

Loveland, Walter; Yao, Larry

2017-11-01

Formally, the cross section for producing a heavy evaporation residue, σEVR, in a fusion reaction can be written as where E is the center of mass energy, and T is the probability of the colliding nuclei to overcome the potential barrier in the entrance channel and reach the contact point. PCN is the probability that the projectile-target system will evolve from the contact point to the compound nucleus. Wsur is the probability that the compound nucleus will decay to produce an evaporation residue rather than fissioning. However, one must remember that the Wsur term effectively sets the allowed values of the spin, which in turn, restricts the values of the capture and fusion cross sections. We point out the implications of this fact for capture cross sections for heavy element formation reactions.

Low spin structure of 86Se: Confirmation of γ collectivity at N =52

NASA Astrophysics Data System (ADS)

Materna, T.; Urban, W.; Sieja, K.; Köster, U.; Faust, H.; Czerwiński, M.; RzÄ ca-Urban, T.; Bernards, C.; Fransen, C.; Jolie, J.; Regis, J.-M.; Thomas, T.; Warr, N.

2015-09-01

The 86Se nucleus has been investigated by γ -ray spectroscopy using an array of Ge detectors placed at the exit of the fission-fragment mass separator Lohengrin of the Institut Laue-Langevin. New transitions have been identified by studying the β decay of 86As. An excitation scheme is proposed and includes a 22+ level at 1399 keV and a possible 3+ level that are well reproduced by shell model calculations with the most recent parametrization. The properties of the excitations indicate a possible onset of γ collectivity in 86Se.

The Effect of Stiffness Parameter on Mass Distribution in Heavy-Ion Induced Fission

NASA Astrophysics Data System (ADS)

Soheyli, Saeed; Khalil Khalili, Morteza; Ashrafi, Ghazaaleh

2018-06-01

The stiffness parameter of the composite system has been studied for several heavy-ion induced fission reactions without the contribution of non-compound nucleus fission events. In this research, determination of the stiffness parameter is based on the comparison between the experimental data on the mass widths of fission fragments and those predicted by the statistical model treatments at the saddle and scission points. Analysis of the results shows that for the induced fission reactions of different targets by the same projectile, the stiffness parameter of the composite system decreases with increasing the fissility parameter, as well as with increasing the mass number of the compound nucleus. This parameter also exhibits a similar behavior for the reactions of a given target induced by different projectiles. As expected, nearly same stiffness values are obtained for different reactions leading to the same compound nucleus.

Reassessment of fission fragment angular distributions from continuum states in the context of transition-state theory

NASA Astrophysics Data System (ADS)

Vaz, Louis C.; Alexander, John M.

1983-07-01

Fission angular distributions have been studied for years and have been treated as classic examples of trasitions-state theory. Early work involving composite nuclei of relatively low excitation energy E ∗ (⪅35 MeV) and spin I (⪅25ħ) gave support to theory and delimited interesting properties of the transitions-state nuclei. More recent research on fusion fission and sequential fission after deeply inelastic reactions involves composite nuclei of much higher energies (⪅200 MeV) and spins (⪅100ħ). Extension of the basic ideas developed for low-spin nuclei requires detailed consideration of the role of these high spins and, in particular, the “spin window” for fussion. We have made empirical correlations of cross sections for evaporation residues and fission in order to get a description of this spin window. A systematic reanalysis has been made for fusion fission induced by H, He and heavier ions. Empirical correlations of K 20 (K 20 = {IeffT }/{h̷2}) are presented along with comparisons of Ieff to moments of inertia for saddle-point nuclei from the rotating liquid drop model. This model gives an excellent guide for the intermidiate spin zone (30⪅ I ⪅65), while strong shell and/or pairing effects are evident for excitations less than ⪅35 MeV. Observations of strong anisotropies for very high-spin systems signal the demise of certain approximation commonly made in the theory, and suggestions are made toward this end.

Influence of primary fragment excitation energy and spin distributions on fission observables

NASA Astrophysics Data System (ADS)

Litaize, Olivier; Thulliez, Loïc; Serot, Olivier; Chebboubi, Abdelaziz; Tamagno, Pierre

2018-03-01

Fission observables in the case of 252Cf(sf) are investigated by exploring several models involved in the excitation energy sharing and spin-parity assignment between primary fission fragments. In a first step the parameters used in the FIFRELIN Monte Carlo code "reference route" are presented: two parameters for the mass dependent temperature ratio law and two constant spin cut-off parameters for light and heavy fragment groups respectively. These parameters determine the initial fragment entry zone in excitation energy and spin-parity (E*, Jπ). They are chosen to reproduce the light and heavy average prompt neutron multiplicities. When these target observables are achieved all other fission observables can be predicted. We show here the influence of input parameters on the saw-tooth curve and we discuss the influence of a mass and energy-dependent spin cut-off model on gamma-rays related fission observables. The part of the model involving level densities, neutron transmission coefficients or photon strength functions remains unchanged.

Fission Reaction Event Yield Algorithm

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hagmann, Christian; Verbeke, Jerome; Vogt, Ramona

FREYA (Fission Reaction Event Yield Algorithm) is a code that simulated the decay of a fissionable nucleus at specified excitation energy. In its present form, FREYA models spontaneous fission and neutron-induced fission up to 20 MeV. It includes the possibility of neutron emission from the nuclear prior to its fussion (nth chance fission).

Dual neutral particle induced transmutation in CINDER2008

NASA Astrophysics Data System (ADS)

Martin, W. J.; de Oliveira, C. R. E.; Hecht, A. A.

2014-12-01

Although nuclear transmutation methods for fission have existed for decades, the focus has been on neutron-induced reactions. Recent novel concepts have sought to use both neutrons and photons for purposes such as active interrogation of cargo to detect the smuggling of highly enriched uranium, a concept that would require modeling the transmutation caused by both incident particles. As photonuclear transmutation has yet to be modeled alongside neutron-induced transmutation in a production code, new methods need to be developed. The CINDER2008 nuclear transmutation code from Los Alamos National Laboratory is extended from neutron applications to dual neutral particle applications, allowing both neutron- and photon-induced reactions for this modeling with a focus on fission. Following standard reaction modeling, the induced fission reaction is understood as a two-part reaction, with an entrance channel to the excited compound nucleus, and an exit channel from the excited compound nucleus to the fission fragmentation. Because photofission yield data-the exit channel from the compound nucleus-are sparse, neutron fission yield data are used in this work. With a different compound nucleus and excitation, the translation to the excited compound state is modified, as appropriate. A verification and validation of these methods and data has been performed. This has shown that the translation of neutron-induced fission product yield sets, and their use in photonuclear applications, is appropriate, and that the code has been extended correctly.

Identification of a triplet pair intermediate in singlet exciton fission in solution

PubMed Central

Stern, Hannah L.; Musser, Andrew J.; Gelinas, Simon; Parkinson, Patrick; Herz, Laura M.; Bruzek, Matthew J.; Anthony, John; Friend, Richard H.; Walker, Brian J.

2015-01-01

Singlet exciton fission is the spin-conserving transformation of one spin-singlet exciton into two spin-triplet excitons. This exciton multiplication mechanism offers an attractive route to solar cells that circumvent the single-junction Shockley–Queisser limit. Most theoretical descriptions of singlet fission invoke an intermediate state of a pair of spin-triplet excitons coupled into an overall spin-singlet configuration, but such a state has never been optically observed. In solution, we show that the dynamics of fission are diffusion limited and enable the isolation of an intermediate species. In concentrated solutions of bis(triisopropylsilylethynyl)[TIPS]—tetracene we find rapid (<100 ps) formation of excimers and a slower (∼10 ns) break up of the excimer to two triplet exciton-bearing free molecules. These excimers are spectroscopically distinct from singlet and triplet excitons, yet possess both singlet and triplet characteristics, enabling identification as a triplet pair state. We find that this triplet pair state is significantly stabilized relative to free triplet excitons, and that it plays a critical role in the efficient endothermic singlet fission process. PMID:26060309

Calculation of multidimensional potential energy surfaces for even-even transuranium nuclei: systematic investigation of the triaxiality effect on the fission barrier

NASA Astrophysics Data System (ADS)

Chai, Qing-Zhen; Zhao, Wei-Juan; Liu, Min-Liang; Wang, Hua-Lei

2018-05-01

Static fission barriers for 95 even-even transuranium nuclei with charge number Z = 94–118 have been systematically investigated by means of pairing self-consistent Woods-Saxon-Strutinsky calculations using the potential energy surface approach in multidimensional (β 2, γ, β 4) deformation space. Taking the heavier 252Cf nucleus (with the available fission barrier from experiment) as an example, the formation of the fission barrier and the influence of macroscopic, shell and pairing correction energies on it are analyzed. The results of the present calculated β 2 values and barrier heights are compared with previous calculations and available experiments. The role of triaxiality in the region of the first saddle is discussed. It is found that the second fission barrier is also considerably affected by the triaxial deformation degree of freedom in some nuclei (e.g., the Z=112–118 isotopes). Based on the potential energy curves, general trends of the evolution of the fission barrier heights and widths as a function of the nucleon numbers are investigated. In addition, the effects of Woods-Saxon potential parameter modifications (e.g., the strength of the spin-orbit coupling and the nuclear surface diffuseness) on the fission barrier are briefly discussed. Supported by National Natural Science Foundation of China (11675148, 11505157), the Project of Youth Backbone Teachers of Colleges and Universities of Henan Province (2017GGJS008), the Foundation and Advanced Technology Research Program of Henan Province (162300410222), the Outstanding Young Talent Research Fund of Zhengzhou University (1521317002) and the Physics Research and Development Program of Zhengzhou University (32410017)

Investigation of the heavy nuclei fission with anomalously high values of the fission fragments total kinetic energy

NASA Astrophysics Data System (ADS)

Khryachkov, Vitaly; Goverdovskii, Andrei; Ketlerov, Vladimir; Mitrofanov, Vecheslav; Sergachev, Alexei

2018-03-01

Binary fission of 232Th and 238U induced by fast neutrons were under intent investigation in the IPPE during recent years. These measurements were performed with a twin ionization chamber with Frisch grids. Signals from the detector were digitized for further processing with a specially developed software. It results in information of kinetic energies, masses, directions and Bragg curves of registered fission fragments. Total statistics of a few million fission events were collected during each experiment. It was discovered that for several combinations of fission fragment masses their total kinetic energy was very close to total free energy of the fissioning system. The probability of such fission events for the fast neutron induced fission was found to be much higher than for spontaneous fission of 252Cf and thermal neutron induced fission of 235U. For experiments with 238U target the energy of incident neutrons were 5 MeV and 6.5 MeV. Close analysis of dependence of fission fragment distribution on compound nucleus excitation energy gave us some explanation of the phenomenon. It could be a process in highly excited compound nucleus which leads the fissioning system from the scission point into the fusion valley with high probability.

Radiochemistry and the Study of Fission

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rundberg, Robert S.

These are slides from a lecture given at UC Berkeley. Radiochemistry has been used to study fission since its discovery. Radiochemical methods are used to determine cumulative mass yields. These measurements have led to the two-mode fission hypothesis to model the neutron energy dependence of fission product yields. Fission product yields can be used for the nuclear forensics of nuclear explosions. The mass yield curve depends on both the fuel and the neutron spectrum of a device. Recent studies have shown that the nuclear structure of the compound nucleus can affect the mass yield distribution. The following topics are covered:more » In the beginning: the discovery of fission; forensics using fission products: what can be learned from fission products, definitions of R-values and Q-values, fission bases, K-factors and fission chambers, limitations; the neutron energy dependence of the mass yield distribution (the two mode fission hypothesis); the influence of nuclear structure on the mass yield distribution. In summary: Radiochemistry has been used to study fission since its discovery. Radiochemical measurement of fission product yields have provided the highest precision data for developing fission models and for nuclear forensics. The two-mode fission hypothesis provides a description of the neutron energy dependence of the mass yield curve. However, data is still rather sparse and more work is needed near second and third chance fission. Radiochemical measurements have provided evidence for the importance of nuclear states in the compound nucleus in predicting the mass yield curve in the resonance region.« less

Advanced model for the prediction of the neutron-rich fission product yields

NASA Astrophysics Data System (ADS)

Rubchenya, V. A.; Gorelov, D.; Jokinen, A.; Penttilä, H.; Äystö, J.

2013-12-01

The consistent models for the description of the independent fission product formation cross sections in the spontaneous fission and in the neutron and proton induced fission at the energies up to 100 MeV is developed. This model is a combination of new version of the two-component exciton model and a time-dependent statistical model for fusion-fission process with inclusion of dynamical effects for accurate calculations of nucleon composition and excitation energy of the fissioning nucleus at the scission point. For each member of the compound nucleus ensemble at the scission point, the primary fission fragment characteristics: kinetic and excitation energies and their yields are calculated using the scission-point fission model with inclusion of the nuclear shell and pairing effects, and multimodal approach. The charge distribution of the primary fragment isobaric chains was considered as a result of the frozen quantal fluctuations of the isovector nuclear matter density at the scission point with the finite neck radius. Model parameters were obtained from the comparison of the predicted independent product fission yields with the experimental results and with the neutron-rich fission product data measured with a Penning trap at the Accelerator Laboratory of the University of Jyväskylä (JYFLTRAP).

High spin states in {sup 151,153}Pr, {sup 157}Sm, and {sup 93}Kr

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hwang, J. K.; Ramayya, A. V.; Hamilton, J. H.

2010-09-15

High spin states are observed for the first time in the neutron-rich nuclei {sup 151,153}Pr, {sup 157}Sm, and {sup 93}Kr from the spontaneous fission of {sup 252}Cf. Twenty new transitions in {sup 151}Pr, twelve in {sup 153}Pr, five in {sup 157}Sm, and four in {sup 93}Kr were identified by using x-ray(Pr/Sm)-{gamma}-{gamma} and {gamma}-{gamma}-{gamma} triple coincidences. From the measured total internal conversion coefficients {alpha}{sub T} of four low-energy transitions in {sup 151,153}Pr, we determine that two bands in each nucleus have opposite parity. The interlacing E1 transitions between the bands suggest a form of parity doubling in {sup 151,153}Pr. New bandsmore » in {sup 157}Sm and {sup 93}Kr are reported. The half-life of the 354.8 keV state in {sup 93}Kr is measured to be 10(2) ns.« less

High-spin states in the N=50 nucleus ^87Rb

NASA Astrophysics Data System (ADS)

Fotiades, N.; Cizewski, J. A.; Krücken, R.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Becker, J. A.; Bernstein, L. A.; McNabb, D. P.; Younes, W.

2001-10-01

High-spin states in ^87Rb have been studied following the fission of two compound nuclei (^199Tl and ^197Pb) formed in different fusion-evaporation reactions. The Gammasphere array at LBNL was used to detect γ-ray coincidences. The level scheme has been extended above the previously known 1578 keV, 9/2^+ isomer by observation of many states up to ~7.2 MeV excitation energy. Coupling of the odd g_9/2 proton to the yrast states in the ^86Kr core accounts for the first excited states observed above the 9/2^+ isomer. The level scheme of ^87Rb is also compared to excitations in ^85Kr and the ^89Y isotone. This work has been supported in part by the U.S. Department of Energy under Contracts No. W-7405-ENG-36 (LANL), FG02-91ER-40609 (Yale), W-7405-ENG-48 (LLNL) and AC03-76SF00098 (LBNL) and by the National Science Foundation (Rutgers).

Statistical prescission point model of fission fragment angular distributions

NASA Astrophysics Data System (ADS)

John, Bency; Kataria, S. K.

1998-03-01

In light of recent developments in fission studies such as slow saddle to scission motion and spin equilibration near the scission point, the theory of fission fragment angular distribution is examined and a new statistical prescission point model is developed. The conditional equilibrium of the collective angular bearing modes at the prescission point, which is guided mainly by their relaxation times and population probabilities, is taken into account in the present model. The present model gives a consistent description of the fragment angular and spin distributions for a wide variety of heavy and light ion induced fission reactions.

Singlet Fission Involves an Interplay between Energetic Driving Force and Electronic Coupling in Perylenediimide Films

DOE PAGES

Le, Aaron K.; Bender, Jon A.; Arias, Dylan H.; ...

2017-12-14

Due to its ability to offset thermalization losses in photoharvesting systems, singlet fission has become a topic of research interest. During singlet fission, a high energy spin-singlet state in an organic semiconductor divides its energy to form two lower energy spin-triplet excitations on neighboring chromophores. While key insights into mechanisms leading to singlet fission have been gained recently, developing photostable compounds that undergo quantitative singlet fission remains a key challenge. In this report, we explore triplet exciton production via singlet fission in films of perylenediimides, a class of compounds with a long history of use as industrial dyes and pigmentsmore » due to their photostability. As singlet fission necessitates electron transfer between neighboring molecules, its rate and yield depend sensitively on their local arrangement. Here, by adding different functional groups at their imide positions, we control how perylenediimides pack in the solid state.« less

Singlet Fission Involves an Interplay between Energetic Driving Force and Electronic Coupling in Perylenediimide Films

DOE Office of Scientific and Technical Information (OSTI.GOV)

Le, Aaron K.; Bender, Jon A.; Arias, Dylan H.

Due to its ability to offset thermalization losses in photoharvesting systems, singlet fission has become a topic of research interest. During singlet fission, a high energy spin-singlet state in an organic semiconductor divides its energy to form two lower energy spin-triplet excitations on neighboring chromophores. While key insights into mechanisms leading to singlet fission have been gained recently, developing photostable compounds that undergo quantitative singlet fission remains a key challenge. In this report, we explore triplet exciton production via singlet fission in films of perylenediimides, a class of compounds with a long history of use as industrial dyes and pigmentsmore » due to their photostability. As singlet fission necessitates electron transfer between neighboring molecules, its rate and yield depend sensitively on their local arrangement. Here, by adding different functional groups at their imide positions, we control how perylenediimides pack in the solid state.« less

Equatorial cavities on asteroids, an evidence of fission events

NASA Astrophysics Data System (ADS)

Tardivel, Simon; Sánchez, Paul; Scheeres, Daniel J.

2018-04-01

This paper investigates the equatorial cavities found on asteroids 2008 EV5 and 2000 DP107 Alpha. As the likelihood of these cavities being impact craters is demonstrated to be low, the paper presents a fission mechanism that explains their existence as a scar of past fission events. The dynamical environment of "top-shaped" asteroids is such that, at high spin rates, an identifiable equatorial region enters into tension before the rest of the body. We propose hypothetical past shapes for 2008 EV5 and 2000 DP107, with mass added within the cavity to recreate a smoother equatorial ridge. The dynamical environment of these hypothetical parent bodies reveal that this modified region is indeed set in tension when spin is increased. The fission process requires tensile strength at the interface between the ejecta and the remaining body, at the moment of fission, between 0 and 2 Pa for 2008 EV5 and between 0 and 15 Pa for 2000 DP107, depending on the precise fission scenario considered. Going back to the spin-up deformation phase of the asteroids, the paper examines how kinetic sieving can form predominantly rocky equators, whose tensile strength could be much lower than that of the rest of the body. This process could explain the low cohesion values implied for this fission mechanism.

Nuclear reactivity control using laser induced polarization

DOEpatents

Bowman, Charles D.

1991-01-01

A control element for reactivity control of a fission source provides an atomic density of .sup.3 He in a control volume which is effective to control criticality as the .sup.3 He is spin-polarized. Spin-polarization of the .sup.3 He affects the cross section of the control volume for fission neutrons and hence, the reactivity. An irradiation source is directed within the .sup.3 He for spin-polarizing the .sup.3 He. An alkali-metal vapor may be included with the .sup.3 He where a laser spin-polarizes the alkali-metal atoms which in turn, spin-couple with .sup.3 He to spin-polarize the .sup.3 He atoms.

Nuclear reactivity control using laser induced polarization

DOEpatents

Bowman, Charles D.

1990-01-01

A control element for reactivity control of a fission source provides an atomic density of .sup.3 He in a control volume which is effective to control criticality as the .sup.3 He is spin-polarized. Spin-polarization of the .sup.3 He affects the cross section of the control volume for fission neturons and hence, the reactivity. An irradiation source is directed within the .sup.3 He for spin-polarizing the .sup.3 He. An alkali-metal vapor may be included with the .sup.3 He where a laser spin-polarizes the alkali-metal atoms which in turn, spin-couple with .sup.3 He to spin-polarize the .sup.3 He atoms.

Monte Carlo based toy model for fission process

NASA Astrophysics Data System (ADS)

Kurniadi, R.; Waris, A.; Viridi, S.

2014-09-01

There are many models and calculation techniques to obtain visible image of fission yield process. In particular, fission yield can be calculated by using two calculations approach, namely macroscopic approach and microscopic approach. This work proposes another calculation approach in which the nucleus is treated as a toy model. Hence, the fission process does not represent real fission process in nature completely. The toy model is formed by Gaussian distribution of random number that randomizes distance likesthe distance between particle and central point. The scission process is started by smashing compound nucleus central point into two parts that are left central and right central points. These three points have different Gaussian distribution parameters such as mean (μCN, μL, μR), and standard deviation (σCN, σL, σR). By overlaying of three distributions, the number of particles (NL, NR) that are trapped by central points can be obtained. This process is iterated until (NL, NR) become constant numbers. Smashing process is repeated by changing σL and σR, randomly.

Nuclear Forensics and Radiochemistry: Fission

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rundberg, Robert S.

Radiochemistry has been used to study fission since it’ discovery. Radiochemical methods are used to determine cumulative mass yields. These measurements have led to the two-mode fission hypothesis to model the neutron energy dependence of fission product yields. Fission product yields can be used for the nuclear forensics of nuclear explosions. The mass yield curve depends on both the fuel and the neutron spectrum of a device. Recent studies have shown that the nuclear structure of the compound nucleus can affect the mass yield distribution.

Quintet multiexciton dynamics in singlet fission

DOE PAGES

Tayebjee, Murad J. Y.; Sanders, Samuel N.; Kumarasamy, Elango; ...

2016-10-17

Singlet fission, in which two triplet excitons are generated from a single absorbed photon, is a key third-generation solar cell concept. Conservation of angular momentum requires that singlet fission populates correlated multiexciton states, which can subsequently dissociate to generate free triplets. However, little is known about electronic and spin correlations in these systems since, due to its typically short lifetime, the multiexciton state is challenging to isolate and study. Here, we use bridged pentacene dimers, which undergo intramolecular singlet fission while isolated in solution and in solid matrices, as a unimolecular model system that can trap long-lived multiexciton states. Wemore » also combine transient absorption and time-resolved electron spin resonance spectroscopies to show that spin correlations in the multiexciton state persist for hundreds of nanoseconds. Furthermore, we confirm long-standing predictions that singlet fission produces triplet pair states of quintet character. Finally, we compare two different pentacene–bridge–pentacene chromophores, systematically tuning the coupling between the pentacenes to understand how differences in molecular structure affect the population and dissociation of multiexciton quintet states.« less

Properties of true quaternary fission of nuclei with allowance for its multistep and sequential character

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kadmensky, S. G., E-mail: kadmensky@phys.vsu.ru; Titova, L. V.; Bulychev, A. O.

An analysis of basicmechanisms of binary and ternary fission of nuclei led to the conclusion that true ternary and quaternary fission of nuclei has a sequential two-step (three-step) character, where, at the first step, a fissile nucleus emits a third light particle (third and fourth light particles) under shakeup effects associated with a nonadiabatic character of its collective deformation motion, whereupon the residual nucleus undergoes fission to two fission fragments. Owing to this, the formulas derived earlier for the widths with respect to sequential two- and three-step decays of nuclei in constructing the theory of two-step twoproton decays and multistepmore » decays in chains of genetically related nuclei could be used to describe the relative yields and angular and energy distributions of third and fourth light particles emitted in (α, α), (t, t), and (α, t) pairs upon the true quaternary spontaneous fission of {sup 252}Cf and thermal-neutron-induced fission of {sup 235}U and {sup 233}U target nuclei. Mechanisms that explain a sharp decrease in the yield of particles appearing second in time and entering into the composition of light-particle pairs that originate from true quaternary fission of nuclei in relation to the yields of analogous particles in true ternary fission of nuclei are proposed.« less

Fission Limit And Surface Disruption Criteria For Asteroids: The Case Of Kleopatra

NASA Astrophysics Data System (ADS)

Hirabayashi, Masatoshi; Scheeres, D. J.

2012-05-01

Asteroid structural failure due to a rapid rotation may occur by two fundamentally different ways: by spinning so fast that surface particles are lofted off due to centripetal accelerations overcoming gravitational attractions or through fission of the body. We generalize these failure modes for real asteroid shapes. How a rubble pile asteroid will fail depends on which of these failure criterion occur first if its spin rate is increased due to the YORP effect, impacts, or planetary flybys. The spin rate at which the interior of an arbitrary uniformly rotating body will undergo tension (and conservatively be susceptible to fission) is computed by taking planar cuts through the shape model, computing the mutual gravitational attraction between the two segments, and determining the spin rate at which the centrifugal force between the two components equals the mutual gravitational attraction. The gravitational attraction computation uses an improved version of the algorithm presented in Werner et al. (2005). To determine the interior point that first undergoes tension, we consider this planar cut perpendicular to the axis of minimum moment of inertia at different cross-sections. On the other hand, we define the surface disruption as follows. For an arbitrary body uniformly rotating at a constant spin rate there are at least four synchronous orbits, which represent circular orbits with the same period as the asteroid spin rate. Surface disruption occurs when the body spins fast enough so that at least one of these synchronous orbits touches the asteroid surface. Kleopatra currently spins with a period of 5.38 hours. The spin period for surface disruption is computed to be 3.02 hours, while the spin period for the interior of the asteroid to go into tension is about 4.8 hours. Thus Kleopatra’s internal fission could occur at spin periods longer than when surface disruption occurs.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tayebjee, Murad J. Y.; Sanders, Samuel N.; Kumarasamy, Elango

Singlet fission, in which two triplet excitons are generated from a single absorbed photon, is a key third-generation solar cell concept. Conservation of angular momentum requires that singlet fission populates correlated multiexciton states, which can subsequently dissociate to generate free triplets. However, little is known about electronic and spin correlations in these systems since, due to its typically short lifetime, the multiexciton state is challenging to isolate and study. Here, we use bridged pentacene dimers, which undergo intramolecular singlet fission while isolated in solution and in solid matrices, as a unimolecular model system that can trap long-lived multiexciton states. Wemore » also combine transient absorption and time-resolved electron spin resonance spectroscopies to show that spin correlations in the multiexciton state persist for hundreds of nanoseconds. Furthermore, we confirm long-standing predictions that singlet fission produces triplet pair states of quintet character. Finally, we compare two different pentacene–bridge–pentacene chromophores, systematically tuning the coupling between the pentacenes to understand how differences in molecular structure affect the population and dissociation of multiexciton quintet states.« less

Gamow-Teller transitions between proton h11/2 and neutron h9/2 partner orbitals in 140I

NASA Astrophysics Data System (ADS)

Moon, B.; Moon, C.-B.; Odahara, A.; Lozeva, R.; Söderström, P.-A.; Nishimura, S.; Yuan, C.; Hong, B.; for theNP1112-RIBF87 Collaboration

2018-04-01

The excited states of the neutron-rich nucleus 140I were, for the first time, investigated by a β-delayed γ-ray spectroscopy. The parent nuclide 140Te was produced through the in-flight fission of the 238U beam at 345 MeV per nucleon on a 9Be target at the Radioactive Isotope Beam Factory (RIBF), RIKEN in Japan. The half-life of 140Te was measured to be 350(5) ms and the spin-parity of ground state of 140I was found to be 2-. The spin-parities of three levels at 926, 1188, and 1787 keV were assigned as 1+ based on log f t values. These allowed Gamow-Teller (G-T) transition-states could be interpreted as the transformation of a neutron in the h9/2 orbital into a proton in the h11/2 orbital. Systematic features of level structures and G-T transitions are discussed in the frameworks of the large-scale shell model and deformed shell model.

Fission foil detector calibrations with high energy protons

NASA Technical Reports Server (NTRS)

Benton, E. V.; Frank, A. L.

1995-01-01

Fission foil detectors (FFD's) are passive devices composed of heavy metal foils in contact with muscovite mica films. The heavy metal nuclei have significant cross sections for fission when irradiated with neutrons and protons. Each isotope is characterized by threshold energies for the fission reactions and particular energy-dependent cross sections. In the FFD's, fission fragments produced by the reactions are emitted from the foils and create latent particle tracks in the adjacent mica films. When the films are processed surface tracks are formed which can be optically counted. The track densities are indications of the fluences and spectra of neutrons and/or protons. In the past, detection efficiencies have been calculated using the low energy neutron calibrated dosimeters and published fission cross sections for neutrons and protons. The problem is that the addition of a large kinetic energy to the (n,nucleus) or (p,nucleus) reaction could increase the energies and ranges of emitted fission fragments and increase the detector sensitivity as compared with lower energy neutron calibrations. High energy calibrations are the only method of resolving the uncertainties in detector efficiencies. At high energies, either proton or neutron calibrations are sufficient since the cross section data show that the proton and neutron fission cross sections are approximately equal. High energy proton beams have been utilized (1.8 and 4.9 GeV, 80 and 140 MeV) for measuring the tracks of fission fragments emitted backward and forward.

Influence of fusion dynamics on fission observables: A multidimensional analysis

NASA Astrophysics Data System (ADS)

Schmitt, C.; Mazurek, K.; Nadtochy, P. N.

2018-01-01

An attempt to unfold the respective influence of the fusion and fission stages on typical fission observables, and namely the neutron prescission multiplicity, is proposed. A four-dimensional dynamical stochastic Langevin model is used to calculate the decay by fission of excited compound nuclei produced in a wide set of heavy-ion collisions. The comparison of the results from such a calculation and experimental data is discussed, guided by predictions of the dynamical deterministic HICOL code for the compound-nucleus formation time. While the dependence of the latter on the entrance-channel properties can straigthforwardly explain some observations, a complex interplay between the various parameters of the reaction is found to occur in other cases. A multidimensional analysis of the respective role of these parameters, including entrance-channel asymmetry, bombarding energy, compound-nucleus fissility, angular momentum, and excitation energy, is proposed. It is shown that, depending on the size of the system, apparent inconsistencies may be deduced when projecting onto specific ordering parameters. The work suggests the possibility of delicate compensation effects in governing the measured fission observables, thereby highlighting the necessity of a multidimensional discussion.

The partial fission of fast spinning asteroids

NASA Astrophysics Data System (ADS)

Tardivel, Simon; Sanchez, Paul; Scheeres, Daniel J.

2016-10-01

The spin rates of asteroids systematically change over time due the Yarkovsky-O'Keefe-Radzievskii-Paddack (YORP) effect. Above a certain spin rate that depends on the body's density, regions of an asteroid can enter in tension, with components held to the body by cohesive forces. When the body fails, deformation or fission can occur. Catastrophic fission leading to complete disruption has been directly observed in active asteroid P/2013 R3. Partial fission, the loss of only part of the body, has been proposed as a mechanism for the formation of binaries and is explored here.The equatorial cavities of (341843) 2008 EV5 and of (185851) 2000 DP107 (a binary system) are consistent with a localized partial fission of the body (LPSC 2016 #1036). The examination of the gravity field of these bodies reveals that a mass placed within these cavities could be shed. In this mechanism, the outward pull of inertial forces creates an average stress at the cavity interface of ≈1 Pa for 2008 EV5 and ≈3 Pa for 2000 DP107 at spin periods of ≈3.15 h for the assumed densities of 1.3 g/cm3.This work continues the study of this partial, localized fission. Specifically, it addresses the issue of the low cohesion necessary to the mechanism. These cohesion values are typically lower than global strength values inferred on other asteroids (10 - 200 Pa), meaning that partial fission may occur prior to larger-scale deformations. Yet, several processes can explain the discrepancy, as they can naturally segregate particles by size. For instance, landslides or granular convection (Brazil nut effect) could bring larger boulders to the equator of the body, while finer particles are left at higher latitudes or sink to the center. Conversely, failure of the interior could bring boulders to the surface. The peculiar profile shape of these asteroids, shared by many binaries (e.g. 1999 KW4, 1996 FG3) may also be a clue of this heterogeneity, as this "spin top" shape is obtained in simulations with a weak shell and a strong core.Using observations and simulations, we consider these processes and the role that this partial fission mechanism could play in the formation of binary asteroids and the creation of equatorial divots on asteroids.

Dynamical approach to heavy-ion induced fusion using actinide target

NASA Astrophysics Data System (ADS)

Aritomo, Y.; Hagino, K.; Chiba, S.; Nishio, K.

2012-10-01

To treat heavy-ion reactions using actinide target nucleus, we propose a model which takes into account the coupling to the collective states of interacting nuclei in the penetration of the Coulomb barrier and the dynamical evolution of nuclear shape from the contact configuration. A fluctuation-dissipation model (Langevin equation) was applied in the dynamical calculation, where effect of nuclear orientation at the initial impact on the prolately deformed target nucleus was considered. Using this model, we analyzed the experimental data for the mass distribution of fission fragments (MDFF) in the reaction of 36S+238U at several incident energies. Fusion-fission, quasifission and deep-quasi-fission are separated as different trajectories on the potential energy surface. We estimated the fusion cross section of the reaction.

Fission fragment mass distributions from 210Po and 213At

NASA Astrophysics Data System (ADS)

Sen, A.; Ghosh, T. K.; Bhattacharya, S.; Banerjee, K.; Bhattacharya, C.; Kundu, S.; Mukherjee, G.; Asgar, A.; Dey, A.; Dhal, A.; Shaikh, Md. Moin; Meena, J. K.; Manna, S.; Pandey, R.; Rana, T. K.; Roy, Pratap; Roy, T.; Srivastava, V.; Bhattacharya, P.

2017-12-01

Background: The influence of shell effect on the dynamics of the fusion fission process and its evolution with excitation energy in the preactinide Hg-Pb region in general is a matter of intense research in recent years. In particular, a strong ambiguity remains for the neutron shell closed 210Po nucleus regarding the role of shell effect in fission around ≈30 -40 MeV of excitation energy. Purpose: We have measured the fission fragment mass distribution of 210Po populated using fusion of 4He+206Pb at different excitation energies and compare the result with recent theoretical predictions as well as with our previous measurement for the same nucleus populated through a different entrance channel. Mass distribution in the fission of the neighboring nuclei 213At is also studied for comparison. Methods: Two large area multiwire proportional counters (MWPC) were used for complete kinematical measurement of the coincident fission fragments. The time of flight differences of the coincident fission fragments were used to directly extract the fission fragment mass distributions. Results: The measured fragment mass distribution for the reactions 4He+206Pb and 4He+209Bi were symmetric and the width of the mass distributions were found to increase monotonically with excitation energy above 36.7 MeV and 32.9 MeV, respectively, indicating the absence of shell effects at the saddle. However, in the fission of 210Po, we find minor deviation from symmetric mass distributions at the lowest excitation energy (30.8 MeV). Conclusion: Persistence of shell effect in fission fragment mass distribution of 210Po was observed at the excitation energy ≈31 MeV as predicted by the theory; at higher excitation energy, however, the present study reaffirms the absence of any shell correction in the fission of 210Po.

Development of a “Fission-proxy” Method for the Measurement of 14-MeV Neutron Fission Yields at CAMS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gharibyan, Narek

2016-10-25

Relative fission yield measurements were made for 50 fission products from 25.6±0.5 MeV alpha-induced fission of Th-232. Quantitative comparison of these experimentally measured fission yields with the evaluated fission yields from 14-MeV neutron-induced fission of U-235 demonstrates the feasibility of the proposed fission-proxy method. This new technique, based on the Bohr-independence hypothesis, permits the measurement of fission yields from an alternate reaction pathway (Th-232 + 25.6 MeV α → U-236* vs. U-235 + 14-MeV n → U-236*) given that the fission process associated with the same compound nucleus is independent of its formation. Other suitable systems that can potentially bemore » investigated in this manner include (but are not limited to) Pu-239 and U-237.« less

Yrast excitations of neutron-rich nuclei around doubly magic Tin-132

NASA Astrophysics Data System (ADS)

Bhattacharyya, Pallab Kumar

Investigation of the yrast structures of neutron-rich nuclei around the double closed shell nucleus 132Sn is important in the understanding of simple two-body nucleon-nucleon interactions in that region. However conventional fusion-evaporation methods do not populate these nuclei and β-decay studies are useful only in studying low spin states. The spectroscopy of these nuclei from thick target γ-γ coincidence measurements of deep inelastic heavy ion collisions as well as from fission fragment γ-ray studies using large multidetector arrays are presented in this thesis. Analyses of data from the 124Sn + 665 MeV 136Xe and 130Te + 272 MeV 64Ni deep inelastic experiments identified new yrast isomers in the N = 80 nuclei 134Xe and 136Ba which de- excite by γ-ray cascades concluding with their known 4+/to2+ and 2+/to0+ transitions. The isomeric decay characteristics are presented and discussed in light of the systematic features in N = 80 isotones. By analyzing fission product γ-ray data measured at Eurogam II using a 248Cm source, yrast level structures of the two-, three- and four-proton N = 82 isotones 134Te, 135I and 136Xe were developed, and the proton-proton interactions from the two-body nucleus 134Te were used in interpreting 135I and 136Xe levels using shell model calculations. From the same data the yrast states in the N = 83 isotones 134Sb, 135Te, 136I and 137Xe were explored, and key proton-neutron interactions were extracted from the 134Sb level spectrum which were used in interpreting the levels of the other N = 83 isotones. Similarly yrast states in previously unexplored N = 81 isotones 132Sb and 133Te were also identified and interpreted with shell model calculations; the 132Sb level spectrum yielded important proton-neutron hole interactions. Neutron core-excited states at higher energies were also identified in most of these nuclei. For establishing isotopic assignments of unknown cascades, the γgamma cross coincidences between heavy and light fission partners were vital. Overall, both deep inelastic and fission product studies have contributed to the exploration of an otherwise inaccessible region of the nuclidic chart. This opens up a new horizon in studying the structure of these important neutron-rich nuclei.

Reexamining the role of the (n ,γ f ) process in the low-energy fission of 235U and 239Pu

NASA Astrophysics Data System (ADS)

Lynn, J. E.; Talou, P.; Bouland, O.

2018-06-01

The (n ,γ f ) process is reviewed in light of modern nuclear reaction calculations in both slow and fast neutron-induced fission reactions on 235U and 239Pu. Observed fluctuations of the average prompt fission neutron multiplicity and average total γ -ray energy below 100-eV incident neutron energy are interpreted in this framework. The surprisingly large contribution of the M 1 transitions to the prefission γ -ray spectrum of 239Pu is explained by the dominant fission probabilities of 0+ and 2+ transition states, which can only be accessed from compound nucleus states formed by the interaction of s -wave neutrons with the target nucleus in its ground state, and decaying through M 1 transitions. The impact of an additional low-lying M 1 scissors mode in the photon strength function is analyzed. We review experimental evidence for fission fragment mass and kinetic-energy fluctuations in the resonance region and their importance in the interpretation of experimental data on prompt neutron data in this region. Finally, calculations are extended to the fast energy range where (n ,γ f ) corrections can account for up to 3% of the total fission cross section and about 20% of the capture cross section.

Coulomb- and Antiferromagnetic-Induced Fission in Doubly Charged Cubelike Fe-S Clusters

NASA Astrophysics Data System (ADS)

Yang, Xin; Wang, Xue-Bin; Niu, Shuqiang; Pickett, Chris J.; Ichiye, Toshiko; Wang, Lai-Sheng

2002-09-01

We report the observation of symmetric fission in doubly charged Fe-S cluster anions, [Fe4S4X4]2- -->2[Fe2S2X2]- (X=Cl,Br), owing to both Coulomb repulsion and antiferromagnetic coupling. Photoelectron spectroscopy shows that both the parent and the fission fragments have similar electronic structures and confirms the inverted energy schemes due to the strong spin polarization of the Fe 3d levels. The current observation provides direct confirmation for the unusual spin couplings in the [Fe4S4X4]2- clusters, which contain two valent-delocalized and ferromagnetically coupled Fe2S2 subunits.

Universal functions of nuclear proximity potential for Skyrme nucleus-nucleus interaction in a semiclassical approach

NASA Astrophysics Data System (ADS)

Gupta, Raj K.; Singh, Dalip; Kumar, Raj; Greiner, Walter

2009-07-01

The universal function of the nuclear proximity potential is obtained for the Skyrme nucleus-nucleus interaction in the semiclassical extended Thomas-Fermi (ETF) approach. This is obtained as a sum of the spin-orbit-density-independent and spin-orbit-density-dependent parts of the Hamiltonian density, since the two terms behave differently, the spin-orbit-density-independent part mainly attractive and the spin-orbit-density-dependent part mainly repulsive. The semiclassical expansions of kinetic energy density and spin-orbit density are allowed up to second order, and the two-parameter Fermi density, with its parameters fitted to experiments, is used for the nuclear density. The universal functions or the resulting nuclear proximity potential reproduce the 'exact' Skyrme nucleus-nucleus interaction potential in the semiclassical approach, within less than ~1 MeV of difference, both at the maximum attraction and in the surface region. An application of the resulting interaction potential to fusion excitation functions shows clearly that the parameterized universal functions of nuclear proximity potential substitute completely the 'exact' potential in the Skyrme energy density formalism based on the semiclassical ETF method, including also the modifications of interaction barriers at sub-barrier energies in terms of modifying the constants of the universal functions.

Singlet-to-triplet intermediates and triplet exciton dynamics in pentacene thinfilms

NASA Astrophysics Data System (ADS)

Thorsmolle, Verner; Korber, Michael; Obergfell, Emanuel; Kuhlman, Thomas; Campbell, Ian; Crone, Brian; Taylor, Antoinette; Averitt, Richard; Demsar, Jure

Singlet-to-triplet fission in organic semiconductors is a spin-conserving multiexciton process in which one spin-zero singlet excitation is converted into two spin-one triplet excitations on an ultrafast timescale. Current scientific interest into this carrier multiplication process is largely driven by prospects of enhancing the efficiency in photovoltaic applications by generating two long-lived triplet excitons by one photon. The fission process is known to involve intermediate states, known as correlated triplet pairs, with an overall singlet character, before being interchanged into uncorrelated triplets. Here we use broadband femtosecond real-time spectroscopy to study the excited state dynamics in pentacene thin films, elucidating the fission process and the role of intermediate triplet states. VKT and AJT acknowledge support by the LDRD program at Los Alamos National Laboratory and the Department of Energy, Grant No. DE-FG02-04ER118. MK, MO and JD acknowledge support by the Alexander von Humboldt Foundation.

The role of spin–rotation coupling in the non-exponential decay of hydrogen-like heavy ions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lambiase, Gaetano, E-mail: lambiase@sa.infn.it; INFN, Sezione di Napoli; International Institute for Advanced Scientific Studies, 89019 Vietri sul Mare

2013-05-15

Recent experiments carried out at the storage ring of GSI in Darmstadt reveal an unexpected oscillation in the orbital electron capture and subsequent decay of hydrogen-like {sup 140}Pr{sup 58+}, {sup 142}Pm{sup 60+} and {sup 122}I{sup 52+}. The modulations have periods of 7.069(8) s, 7.10(22) s and 6.1 s respectively in the laboratory frame and are superimposed on the expected exponential decays. In this paper we propose a semiclassical model in which the observed modulations arise from the coupling of rotation to the spins of electron and nucleus. We show that the modulations are connected to quantum beats and to themore » effect of the Thomas precession on the spins of bound electron and nucleus, the magnetic moment precessions of electron and nucleus and their cyclotron frequencies. We also show that the spin–spin coupling of electron and nucleus, though dominant relative to the magnetic moment coupling of electron and nucleus with the storage ring magnetic field, does not contribute to the modulation because these terms average out during the time of flight of the ions, or cancel out. The model also predicts that the anomaly cannot be observed if the motion of the ions is rectilinear, or if the ions are stopped in a target (decay of neutral atoms in solid environments). It also supports the notion that no modulation occurs for the β{sup +}-decay branch. -- Highlights: ► Spin precession of the spin of nucleus and electron in storage ring. ► Coupling of rotation to the spin of electron and nucleus. ► Modulation in the decay probability of the heavy ions induced by quantum beats. ► Comparison with experimental data.« less

Point-by-point model calculation of the prompt neutron multiplicity distribution ν(A) in the incident neutron energy range of multi-chance fission

NASA Astrophysics Data System (ADS)

Tudora, Anabella; Hambsch, Franz-Josef; Tobosaru, Viorel

2017-09-01

Prompt neutron multiplicity distributions ν(A) are required for prompt emission correction of double energy (2E) measurements of fission fragments to determine pre-neutron fragment properties. The lack of experimental ν(A) data especially at incident neutron energies (En) where the multi-chance fission occurs impose the use of ν(A) predicted by models. The Point-by-Point model of prompt emission is able to provide the individual ν(A) of the compound nuclei of the main and secondary nucleus chains undergoing fission at a given En. The total ν(A) is obtained by averaging these individual ν(A) over the probabilities of fission chances (expressed as total and partial fission cross-section ratios). An indirect validation of the total ν(A) results is proposed. At high En, above 70 MeV, the PbP results of individual ν(A) of the first few nuclei of the main and secondary nucleus chains exhibit an almost linear increase. This shape is explained by the damping of shell effects entering the super-fluid expression of the level density parameters. They tend to approach the asymptotic values for most of the fragments. This fact leads to a smooth and almost linear increase of fragment excitation energy with the mass number that is reflected in a smooth and almost linear behaviour of ν(A).

Reexamining the role of the ( n , γ f ) process in the low-energy fission of U 235 and Pu 239

DOE PAGES

Lynn, J. E.; Talou, P.; Bouland, O.

2018-06-01

In this paper, themore » $$(n,{\\gamma}f)$$ process is reviewed in light of modern nuclear reaction calculations in both slow and fast neutron-induced fission reactions on $$^{235}\\mathrm{U}$$ and $$^{239}\\mathrm{Pu}$$. Observed fluctuations of the average prompt fission neutron multiplicity and average total $${\\gamma}$$-ray energy below 100-eV incident neutron energy are interpreted in this framework. The surprisingly large contribution of the $M1$ transitions to the prefission $${\\gamma}$$-ray spectrum of $$^{239}\\mathrm{Pu}$$ is explained by the dominant fission probabilities of $${0}^{+}$$ and $${2}^{+}$$ transition states, which can only be accessed from compound nucleus states formed by the interaction of $s$-wave neutrons with the target nucleus in its ground state, and decaying through $M1$ transitions. The impact of an additional low-lying $M1$ scissors mode in the photon strength function is analyzed. We review experimental evidence for fission fragment mass and kinetic-energy fluctuations in the resonance region and their importance in the interpretation of experimental data on prompt neutron data in this region. In conclusion, calculations are extended to the fast energy range where $$(n,{\\gamma}f)$$ corrections can account for up to 3% of the total fission cross section and about 20% of the capture cross section.« less

Reexamining the role of the ( n , γ f ) process in the low-energy fission of U 235 and Pu 239

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lynn, J. E.; Talou, P.; Bouland, O.

In this paper, themore » $$(n,{\\gamma}f)$$ process is reviewed in light of modern nuclear reaction calculations in both slow and fast neutron-induced fission reactions on $$^{235}\\mathrm{U}$$ and $$^{239}\\mathrm{Pu}$$. Observed fluctuations of the average prompt fission neutron multiplicity and average total $${\\gamma}$$-ray energy below 100-eV incident neutron energy are interpreted in this framework. The surprisingly large contribution of the $M1$ transitions to the prefission $${\\gamma}$$-ray spectrum of $$^{239}\\mathrm{Pu}$$ is explained by the dominant fission probabilities of $${0}^{+}$$ and $${2}^{+}$$ transition states, which can only be accessed from compound nucleus states formed by the interaction of $s$-wave neutrons with the target nucleus in its ground state, and decaying through $M1$ transitions. The impact of an additional low-lying $M1$ scissors mode in the photon strength function is analyzed. We review experimental evidence for fission fragment mass and kinetic-energy fluctuations in the resonance region and their importance in the interpretation of experimental data on prompt neutron data in this region. In conclusion, calculations are extended to the fast energy range where $$(n,{\\gamma}f)$$ corrections can account for up to 3% of the total fission cross section and about 20% of the capture cross section.« less

Dynamical approach to fusion-fission process in superheavy mass region

NASA Astrophysics Data System (ADS)

Aritomo, Y.; Hinde, D. J.; Wakhle, A.; du Rietz, R.; Dasgupta, M.; Hagino, K.; Chiba, S.; Nishio, K.

2012-10-01

In order to describe heavy-ion fusion reactions around the Coulomb barrier with an actinide target nucleus, we propose a model which combines the coupled-channels approach and a fluctuation-dissipation model for dynamical calculations. This model takes into account couplings to the collective states of the interacting nuclei in the penetration of the Coulomb barrier and the subsequent dynamical evolution of a nuclear shape from the contact configuration. In the fluctuation-dissipation model with a Langevin equation, the effect of nuclear orientation at the initial impact on the prolately deformed target nucleus is considered. Fusion-fission, quasifission and deep quasifission are separated as different Langevin trajectories on the potential energy surface. Using this model, we analyze the experimental data for the mass distribution of fission fragments (MDFF) in the reaction of 36S+238U at several incident energies around the Coulomb barrier.

Fission Barrier of ^254No at High Spin

NASA Astrophysics Data System (ADS)

Henning, G.; Khoo, T. L.; Seweryniak, D.; Back, B. B.; Bertone, P. F.; Carpenter, M. P.; Greene, J. P.; Gürdal, G.; Hoffman, C. R.; Janssens, R. V. F.; Kay, B. P.; Kondev, F. G.; Lauritsen, T.; Lister, C. J.; McCutchan, E. A.; Nair, C.; Rogers, A. M.; Zhu, S.; Chiara, C. J.; Hauschild, K.; Lopez-Martens, A.; Heinz, A.; Piot, J.; Chowdhury, P.; Lakshmi, S.

2010-11-01

Superheavy nuclei provide opportunities to study nuclear structure at the limits in charge, spin and excitation energy. These nuclei exist only because shell effects create a fission barrier Bf. Hence, it is important to determine Bf and its spin dependence. For ^254No, the maximum spin and energy were found [1] to be Imax= 22 and E* = 8 MeV in the reaction ^208Pb(^48Ca,2n) at a beam energy of 219 MeV. At 223 MeV, the maximum spin increases to 32. In contrast, the spin in ^220Th, produced [2] in the ^176Yb(^48 Ca,4n) reaction at 206 and 219 MeV, saturates at 20. A measurement of the entry distribution of ^254No at 223 MeV has been performed to determine Bf(I) and results will be reported.[4pt] [1] P. Reiter et al., Phys. Rev. Lett. 84, 3542 (2000).[0pt] [2] A. Heinz et al., Nucl. Phys. A682, 458c (2001)

Study of heavy-ion induced fission for heavy-element synthesis

NASA Astrophysics Data System (ADS)

Nishio, K.; Ikezoe, H.; Hofmann, S.; Heßberger, F. P.; Ackermann, D.; Antalic, S.; Aritomo, Y.; Comas, V. F.; Düllman, Ch. E.; Gorshkov, A.; Graeger, R.; Heinz, S.; Heredia, J. A.; Hirose, K.; Khuyagbaatar, J.; Kindler, B.; Kojouharov, I.; Lommel, B.; Makii, H.; Mann, R.; Mitsuoka, S.; Nagame, Y.; Nishinaka, I.; Ohtsuki, T.; Popeko, A. G.; Saro, S.; Schädel, M.; Türler, A.; Wakabayashi, Y.; Watanabe, Y.; Yakushev, A.; Yeremin, A. V.

2014-03-01

Fission fragment mass distributions were measured in heavy-ion induced fissions using 238U target nucleus. The measured mass distributions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and qasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their incident energy dependence. Fusion probability was determined in the analysis, and the values were consistent with those determined from the evaporation residue cross sections.

Parallel theoretical study of the two components of the prompt fission neutrons: Dynamically released at scission and evaporated from fully accelerated fragments

NASA Astrophysics Data System (ADS)

Carjan, Nicolae; Rizea, Margarit; Talou, Patrick

2017-09-01

Prompt fission neutrons (PFN) angular and energy distributions for the reaction 235U(nth,f) are calculated as a function of the mass asymmetry of the fission fragments using two extreme assumptions: 1) PFN are released during the neck rupture due to the diabatic coupling between the neutron degree of freedom and the rapidly changing neutron-nucleus potential. These unbound neutrons are faster than the separation of the nascent fragments and most of them leave the fissioning system in few 10-21 sec. i.e., at the begining of the acceleration phase. Surrounding the fissioning nucleus by a sphere one can calculate the radial component of the neutron current density. Its time integral gives the angular distribution with respect to the fission axis. The average energy of each emitted neutron is also calculated using the unbound part of each neutron wave packet. The distribution of these average energies gives the general trends of the PFN spectrum: the slope, the range and the average value. 2) PFN are evaporated from fully accelerated, fully equilibrated fission fragments. To follow the de-excitation of these fragments via neutron and γ-ray sequential emissions, a Monte Carlo sampling of the initial conditions and a Hauser-Feshbach statistical approach is used. Recording at each step the emission probability, the energy and the angle of each evaporated neutron one can construct the PFN energy and the PFN angular distribution in the laboratory system. The predictions of these two methods are finally compared with recent experimental results obtained for a given fragment mass ratio.

Fission in the landscape of heaviest elements: Some recent examples

NASA Astrophysics Data System (ADS)

Khuyagbaatar, J.; Yakushev, A.; Düllmann, Ch. E.; Ackermann, D.; Andersson, L.-L.; Block, M.; Brand, H.; Even, J.; Forsberg, U.; Hartmann, W.; Herzberg, R.-D.; Heßberger, F. P.; Hoffmann, J.; Hübner, A.; Jäger, E.; Jeppsson, J.; Kindler, B.; Kratz, J. V.; Krier, J.; Kurz, N.; Lommel, B.; Maiti, M.; Minami, S.; Rudolph, D.; Runke, J.; Sarmiento, L. G.; Schädel, M.; Schausten, B.; Steiner, J.; Heidenreich, T. Torres De; Uusitalo, J.; Wiehl, N.; Yakusheva, V.

2016-12-01

The fission process still remains a main factor that determines the stability of the atomic nucleus of heaviest elements. Fission half-lives vary over a wide range, 10-19-1024 s. Present experimental techniques for the synthesis of the superheavy elements that usually measure α-decay chains are sensitive only in a limited range of half-lives, often 10-5-103 s. In the past years, measurement techniques for very short-lived and very long-lived nuclei were significantly improved at the gas-filled recoil separator TASCA at GSI Darmstadt. Recently, several experimental studies of fission-related phenomena have successfully been performed. In this paper, results on 254-256Rf and 266Lr are presented and corresponding factors for retarding the fission process are discussed.

Dynamics of rotationally fissioned asteroids: Source of observed small asteroid systems

NASA Astrophysics Data System (ADS)

Jacobson, Seth A.; Scheeres, Daniel J.

2011-07-01

We present a model of near-Earth asteroid (NEA) rotational fission and ensuing dynamics that describes the creation of synchronous binaries and all other observed NEA systems including: doubly synchronous binaries, high- e binaries, ternary systems, and contact binaries. Our model only presupposes the Yarkovsky-O'Keefe-Radzievskii-Paddack (YORP) effect, "rubble pile" asteroid geophysics, and gravitational interactions. The YORP effect torques a "rubble pile" asteroid until the asteroid reaches its fission spin limit and the components enter orbit about each other (Scheeres, D.J. [2007]. Icarus 189, 370-385). Non-spherical gravitational potentials couple the spin states to the orbit state and chaotically drive the system towards the observed asteroid classes along two evolutionary tracks primarily distinguished by mass ratio. Related to this is a new binary process termed secondary fission - the secondary asteroid of the binary system is rotationally accelerated via gravitational torques until it fissions, thus creating a chaotic ternary system. The initially chaotic binary can be stabilized to create a synchronous binary by components of the fissioned secondary asteroid impacting the primary asteroid, solar gravitational perturbations, and mutual body tides. These results emphasize the importance of the initial component size distribution and configuration within the parent asteroid. NEAs may go through multiple binary cycles and many YORP-induced rotational fissions during their approximately 10 Myr lifetime in the inner Solar System. Rotational fission and the ensuing dynamics are responsible for all NEA systems including the most commonly observed synchronous binaries.

Formation and distribution of fragments in the spontaneous fission of 240Pu

NASA Astrophysics Data System (ADS)

Sadhukhan, Jhilam; Zhang, Chunli; Nazarewicz, Witold; Schunck, Nicolas

2017-12-01

Background: Fission is a fundamental decay mode of heavy atomic nuclei. The prevalent theoretical approach is based on mean-field theory and its extensions where fission is modeled as a large amplitude motion of a nucleus in a multidimensional collective space. One of the important observables characterizing fission is the charge and mass distribution of fission fragments. Purpose: The goal of this Rapid Communication is to better understand the structure of fission fragment distributions by investigating the competition between the static structure of the collective manifold and the stochastic dynamics. In particular, we study the characteristics of the tails of yield distributions, which correspond to very asymmetric fission into a very heavy and a very light fragment. Methods: We use the stochastic Langevin framework to simulate the nuclear evolution after the system tunnels through the multidimensional potential barrier. For a representative sample of different initial configurations along the outer turning-point line, we define effective fission paths by computing a large number of Langevin trajectories. We extract the relative contribution of each such path to the fragment distribution. We then use nucleon localization functions along effective fission pathways to analyze the characteristics of prefragments at prescission configurations. Results: We find that non-Newtonian Langevin trajectories, strongly impacted by the random force, produce the tails of the fission fragment distribution of 240Pu. The prefragments deduced from nucleon localizations are formed early and change little as the nucleus evolves towards scission. On the other hand, the system contains many nucleons that are not localized in the prefragments even near the scission point. Such nucleons are distributed rapidly at scission to form the final fragments. Fission prefragments extracted from direct integration of the density and from the localization functions typically differ by more than 30 nucleons even near scission. Conclusions: Our Rapid Communication shows that only theoretical models of fission that account for some form of stochastic dynamics can give an accurate description of the structure of fragment distributions. In particular, it should be nearly impossible to predict the tails of these distributions within the standard formulation of time-dependent density-functional theory. At the same time, the large number of nonlocalized nucleons during fission suggests that adiabatic approaches where the interplay between intrinsic excitations and collective dynamics is neglected are ill suited to describe fission fragment properties, in particular, their excitation energy.

Elastic and inelastic scattering of neutrons on 238U nucleus

NASA Astrophysics Data System (ADS)

Capote, R.; Trkov, A.; Sin, M.; Herman, M. W.; Soukhovitskiĩ, E. Sh.

2014-04-01

Advanced modelling of neutron induced reactions on the 238U nucleus is aimed at improving our knowledge of neutron scattering. Capture and fission channels are well constrained by available experimental data and neutron standard evaluation. A focus of this contribution is on elastic and inelastic scattering cross sections. The employed nuclear reaction model includes - a new rotational-vibrational dispersive optical model potential coupling the low-lying collective bands of vibrational character observed in even-even actinides; - the Engelbrecht-Weidenmüller transformation allowing for inclusion of compound-direct interference effects; - and a multi-humped fission barrier with absorption in the secondary well described within the optical model for fission. Impact of the advanced modelling on elastic and inelastic scattering cross sections including angular distributions and emission spectra is assessed both by comparison with selected microscopic experimental data and integral criticality benchmarks including measured reaction rates (e.g. JEMIMA, FLAPTOP and BIG TEN). Benchmark calculations provided feedback to improve the reaction modelling. Improvement of existing libraries will be discussed.

Dynamics of Db isotopes formed in reactions induced by 238U, 248Cm, and 249Bk across the Coulomb barrier

NASA Astrophysics Data System (ADS)

Kaur, Gurjit; Sandhu, Kirandeep; Kaur, Amandeep; Sharma, Manoj K.

2018-05-01

The dynamical cluster decay model is employed to investigate the decay of *265Db and *267Db nuclei, formed in the 27Al+238U , 18O+249Bk , and 19F+248Cm hot fusion reactions at energies around the Coulomb barrier. First, the fission dynamics of the 27Al+238U reaction is explored by investigating the fragmentation and preformation yield of the reaction. The symmetric mass distribution of the fission fragments is observed for *265Db nucleus, when static β2 i deformations are used within hot optimum orientation approach. However, the mass split gets broaden for the use of β2 i-dynamical hot configuration of the fragments and becomes clearly asymmetric for the cold-static-deformed approach. Within the application of cold orientations of fragments, a new fission channel is observed at mass asymmetry η =0.29 . In addition to 238U-induced reaction, the work is carried out to address the fission and neutron evaporation cross sections of *267Db nucleus formed via 19F+248Cm and 18O+249Bk reactions, besides a comprehensive analysis of fusion and capture processes. Higher fusion cross sections and compound nucleus formation probabilities (PCN) are obtained for the 18O+249Bk reaction, as larger mass asymmetry in the entrance channel leads to reduced Coulomb factor. Finally, the role of sticking (IS) and nonsticking (INS) moments of inertia is analyzed for the 4 n and 5 n channels of *267Db nuclear system.

Microscopic description of fission properties for r-process nuclei

NASA Astrophysics Data System (ADS)

Giuliani, S. A.; Martínez-Pinedo, G.; Robledo, L. M.

2018-01-01

Fission properties of 886 even-even nuclei in the region 84 ≤ Z ≤ 120 and 118 ≤ Z ≤ 250 were computed using the Barcelona-Catania-Paris-Madrid energy density functional. An extensive study of both the potential energy surfaces and collectives inertias was performed. Spontaneous fission half-lives are computed using the semiclassical Wentzel-Kramers-Brillouin formalism. By comparing these three quantities we found that the stability of the nucleus against the fission process is driven by the interplay between both the potential energy and the collective inertias. In our calculations, nuclei with relative long half-lives were found in two regions around Z = 120, N = 182 and Z = 104, N = 222.

Fission Fragment Mass Distributions and Total Kinetic Energy Release of 235-Uranium and 238-Uranium in Neutron-Induced Fission at Intermediate and Fast Neutron Energies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Duke, Dana Lynn

2015-11-12

This Ph.D. dissertation describes a measurement of the change in mass distributions and average total kinetic energy (TKE) release with increasing incident neutron energy for fission of 235U and 238U. Although fission was discovered over seventy-five years ago, open questions remain about the physics of the fission process. The energy of the incident neutron, En, changes the division of energy release in the resulting fission fragments, however, the details of energy partitioning remain ambiguous because the nucleus is a many-body quantum system. Creating a full theoretical model is difficult and experimental data to validate existing models are lacking. Additional fissionmore » measurements will lead to higher-quality models of the fission process, therefore improving applications such as the development of next-generation nuclear reactors and defense. This work also paves the way for precision experiments such as the Time Projection Chamber (TPC) for fission cross section measurements and the Spectrometer for Ion Determination in Fission (SPIDER) for precision mass yields.« less

SPY: A new scission point model based on microscopic ingredients to predict fission fragments properties

NASA Astrophysics Data System (ADS)

Lemaître, J.-F.; Dubray, N.; Hilaire, S.; Panebianco, S.; Sida, J.-L.

2013-12-01

Our purpose is to determine fission fragments characteristics in a framework of a scission point model named SPY for Scission Point Yields. This approach can be considered as a theoretical laboratory to study fission mechanism since it gives access to the correlation between the fragments properties and their nuclear structure, such as shell correction, pairing, collective degrees of freedom, odd-even effects. Which ones are dominant in final state? What is the impact of compound nucleus structure? The SPY model consists in a statistical description of the fission process at the scission point where fragments are completely formed and well separated with fixed properties. The most important property of the model relies on the nuclear structure of the fragments which is derived from full quantum microscopic calculations. This approach allows computing the fission final state of extremely exotic nuclei which are inaccessible by most of the fission model available on the market.

Kinesin-8 Motors Improve Nuclear Centering by Promoting Microtubule Catastrophe

NASA Astrophysics Data System (ADS)

Glunčić, Matko; Maghelli, Nicola; Krull, Alexander; Krstić, Vladimir; Ramunno-Johnson, Damien; Pavin, Nenad; Tolić, Iva M.

2015-02-01

In fission yeast, microtubules push against the cell edge, thereby positioning the nucleus in the cell center. Kinesin-8 motors regulate microtubule catastrophe; however, their role in nuclear positioning is not known. Here we develop a physical model that describes how kinesin-8 motors affect nuclear centering by promoting a microtubule catastrophe. Our model predicts the improved centering of the nucleus in the presence of motors, which we confirmed experimentally in living cells. The model also predicts a characteristic time for the recentering of a displaced nucleus, which is supported by our experiments where we displaced the nucleus using optical tweezers.

Compound Nucleus Reactions in LENR, Analogy to Uranium Fission

NASA Astrophysics Data System (ADS)

Hora, Heinrich; Miley, George; Philberth, Karl

2008-03-01

The discovery of nuclear fission by Hahn and Strassmann was based on a very rare microanalytical result that could not initially indicate the very complicated details of this most important process. A similarity is discussed for the low energy nuclear reactions (LENRs) with analogies to the yield structure found in measurements of uranium fission. The LENR product distribution measured earlier in a reproducible way in experiments with thin film electrodes and a high density deuteron concentration in palladium has several striking similarities with the uranium fission fragment yield curve.ootnotetextG.H. Miley and J.A. Patterson, J. New Energy 1, 11 (1996); G.H. Miley et al, Proc ICCF6, p. 629 (1997).This comparison is specifically focussed to the Maruhn-Greiner local maximum of the distribution within the large-scale minimum when the fission nuclei are excited. Implications for uranium fission are discussed in comparison with LENR relative to the identification of fission a hypothetical compound nuclear reaction via a element ^306X126 with double magic numbers.

Robust singlet fission in pentacene thin films with tuned charge transfer interactions.

PubMed

Broch, K; Dieterle, J; Branchi, F; Hestand, N J; Olivier, Y; Tamura, H; Cruz, C; Nichols, V M; Hinderhofer, A; Beljonne, D; Spano, F C; Cerullo, G; Bardeen, C J; Schreiber, F

2018-03-05

Singlet fission, the spin-allowed photophysical process converting an excited singlet state into two triplet states, has attracted significant attention for device applications. Research so far has focused mainly on the understanding of singlet fission in pure materials, yet blends offer the promise of a controlled tuning of intermolecular interactions, impacting singlet fission efficiencies. Here we report a study of singlet fission in mixtures of pentacene with weakly interacting spacer molecules. Comparison of experimentally determined stationary optical properties and theoretical calculations indicates a reduction of charge-transfer interactions between pentacene molecules with increasing spacer molecule fraction. Theory predicts that the reduced interactions slow down singlet fission in these blends, but surprisingly we find that singlet fission occurs on a timescale comparable to that in pure crystalline pentacene. We explain the observed robustness of singlet fission in such mixed films by a mechanism of exciton diffusion to hot spots with closer intermolecular spacings.

An Act of Scientific Creativity: Meitner, Frisch, and Nuclear Fission

NASA Astrophysics Data System (ADS)

Stuewer, Roger H.

2002-04-01

The dominant event that lay in the background to Werner Heisenberg's fateful meeting with Niels Bohr in occupied Copenhagen in September 1941 was the discovery and interpretation of nuclear fission three years earlier. Michael Frayn has explored that meeting in his play "Copenhagen" in an act of extraordinary literary creativity. In this talk I will explore Lise Meitner's and Otto Robert Frisch's interpretation of nuclear fission as an act of extraordinary scientific creativity. My aim is to understand historically how it was possible for Meitner and Frisch, and only Meitner and Frisch, to arrive at their interpretation as they talked and walked in the snow in the small Swedish village of Kungälv over the Christmas holidays in December 1938. This will require us to examine the history of the liquid-drop model of the nucleus over the preceding decade, from George Gamow's conception of that model in 1928, through Heisenberg and Carl Friedrich von Weizsäcker's extension of it between 1933 and 1936, and finally through Bohr's use of it in his theory of the compound nucleus between 1936 and 1938. We will see how Meitner and Frisch combined their different knowledge of these developments creatively to arrive at their momentous interpretation of nuclear fission.

Fission fragment angular distributions in the reactions {sup 16}O+{sup 188}Os and {sup 28}Si+{sup 176}Yb

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tripathi, R.; Sudarshan, K.; Sharma, S. K.

2009-06-15

Fission fragment angular distributions have been measured in the reactions {sup 16}O+{sup 188}Os and {sup 28}Si+{sup 176}Yb to investigate the contribution from noncompound nucleus fission. Parameters for statistical model calculations were fixed using fission cross section data in the {sup 16}O+{sup 188}Os reaction. Experimental anisotropies were in reasonable agreement with those calculated using the statistical saddle point model for both reactions. The present results are also consistent with those of mass distribution studies in the fission of {sup 202}Po, formed in the reactions with varying entrance channel mass asymmetry. However, the present studies do not show a large fusion hindrancemore » as reported in the pre-actinide region based on the measurement of evaporation residue cross section.« less

Dynamic approach to description of entrance channel effects in angular distributions of fission fragments

NASA Astrophysics Data System (ADS)

Eremenko, D. O.; Drozdov, V. A.; Fotina, O. V.; Platonov, S. Yu.; Yuminov, O. A.

2016-07-01

Background: It is well known that the anomalous behavior of angular anisotropies of fission fragments at sub- and near-barrier energies is associated with a memory of conditions in the entrance channel of the heavy-ion reactions, particularly, deformations and spins of colliding nuclei that determine the initial distributions for the components of the total angular momentum over the symmetry axis of the fissioning system and the beam axis. Purpose: We develop a new dynamic approach, which allows the description of the memory effects in the fission fragment angular distributions and provides new information on fusion and fission dynamics. Methods: The approach is based on the dynamic model of the fission fragment angular distributions which takes into account stochastic aspects of nuclear fission and thermal fluctuations for the tilting mode that is characterized by the projection of the total angular momentum onto the symmetry axis of the fissioning system. Another base of our approach is the quantum mechanical method to calculate the initial distributions over the components of the total angular momentum of the nuclear system immediately following complete fusion. Results: A method is suggested for calculating the initial distributions of the total angular momentum projection onto the symmetry axis for the nuclear systems formed in the reactions of complete fusion of deformed nuclei with spins. The angular distributions of fission fragments for the 16O+232Th,12C+235,236,238, and 13C+235U reactions have been analyzed within the dynamic approach over a range of sub- and above-barrier energies. The analysis allowed us to determine the relaxation time for the tilting mode and the fraction of fission events occurring in times not larger than the relaxation time for the tilting mode. Conclusions: It is shown that the memory effects play an important role in the formation of the angular distributions of fission fragments for the reactions induced by heavy ions. The approach developed for analysis of the effects is a suitable tool to get insight into the complete fusion-fission dynamics, in particular, to investigate the mechanism of the complete fusion and fission time scale.

Oxidative metabolism of phenanthrene and anthracene by soil pseudomonads. The ring-fission mechanism

PubMed Central

Evans, W. C.; Fernley, H. N.; Griffiths, E.

1965-01-01

1. Phenanthrene is oxidatively metabolized by soil pseudomonads through trans-3,4-dihydro-3,4-dihydroxyphenanthrene to 3,4-dihydroxyphenanthrene, which then undergoes cleavage. 2. Some properties of the ring-fission product, cis-4-(1-hydroxynaphth-2-yl)-2-oxobut-3-enoic acid, are described. The Fe2+-dependent oxygenase therefore disrupts the bond between C-4 and the angular C of the phenanthrene nucleus. 3. An enzyme of the aldolase type converts the fission product into 1-hydroxy-2-naphthaldehyde (2-formyl-1-hydroxynaphthalene). An NAD-specific dehydrogenase is also present in the cell-free extract, which oxidizes the aldehyde to 1-hydroxy-2-naphthoic acid. This is then oxidatively decarboxylated to 1,2-dihydroxynaphthalene, thus allowing continuation of metabolism via the naphthalene pathway. 4. Anthracene is similarly metabolized, through 1,2-dihydro-1,2-dihydroxyanthracene to 1,2-dihydroxyanthracene, in which ring-fission occurs to give cis-4-(2-hydroxynaphth-3-yl)-2-oxobut-3-enoic acid. The position of cleavage is again at the bond between the angular C and C-1 of the anthracene nucleus. 5. Enzymes that convert the fission product through 2-hydroxy-3-naphthaldehyde into 2-hydroxy-3-naphthoic acid were demonstrated. The further metabolism of this acid is discussed. 6. The Fe2+-dependent oxygenase responsible for cleavage of all the o-dihydroxyphenol derivatives appears to be catechol 2,3-oxygenase, and is a constitutive enzyme in the Pseudomonas strains used. PMID:14342521

High-spin structure of 134Xe

NASA Astrophysics Data System (ADS)

Vogt, A.; Birkenbach, B.; Reiter, P.; Blazhev, A.; Siciliano, M.; Valiente-Dobón, J. J.; Wheldon, C.; Bazzacco, D.; Bowry, M.; Bracco, A.; Bruyneel, B.; Chakrawarthy, R. S.; Chapman, R.; Cline, D.; Corradi, L.; Crespi, F. C. L.; Cromaz, M.; de Angelis, G.; Eberth, J.; Fallon, P.; Farnea, E.; Fioretto, E.; Freeman, S. J.; Gadea, A.; Geibel, K.; Gelletly, W.; Gengelbach, A.; Giaz, A.; Görgen, A.; Gottardo, A.; Hayes, A. B.; Hess, H.; Hua, H.; John, P. R.; Jolie, J.; Jungclaus, A.; Korten, W.; Lee, I. Y.; Leoni, S.; Liang, X.; Lunardi, S.; Macchiavelli, A. O.; Menegazzo, R.; Mengoni, D.; Michelagnoli, C.; Mijatović, T.; Montagnoli, G.; Montanari, D.; Napoli, D.; Pearson, C. J.; Pellegri, L.; Podolyák, Zs.; Pollarolo, G.; Pullia, A.; Radeck, F.; Recchia, F.; Regan, P. H.; Şahin, E.; Scarlassara, F.; Sletten, G.; Smith, J. F.; Söderström, P.-A.; Stefanini, A. M.; Steinbach, T.; Stezowski, O.; Szilner, S.; Szpak, B.; Teng, R.; Ur, C.; Vandone, V.; Ward, D.; Warner, D. D.; Wiens, A.; Wu, C. Y.

2016-05-01

Detailed spectroscopic information on the N ˜82 nuclei is necessary to benchmark shell-model calculations in the region. The nuclear structure above long-lived isomers in 134Xe is investigated after multinucleon transfer (MNT) and actinide fission. Xenon-134 was populated as (i) a transfer product in 238U+ 136Xe and 208Pb+ 136Xe MNT reactions and (ii) as a fission product in the 238U+ 136Xe reaction employing the high-resolution Advanced Gamma Tracking Array (AGATA). Trajectory reconstruction has been applied for the complete identification of beamlike transfer products with the magnetic spectrometer PRISMA. The 198Pt 136Xe MNT reaction was studied with the γ -ray spectrometer GAMMASPHERE in combination with the gas detector array Compact Heavy Ion Counter (CHICO). Several high-spin states in 134Xe on top of the two long-lived isomers are discovered based on γ γ -coincidence relationships and information on the γ -ray angular distributions as well as excitation energies from the total kinetic energy loss and fission fragments. The revised level scheme of 134Xe is extended up to an excitation energy of 5.832 MeV with tentative spin-parity assignments up to 16+. Previous assignments of states above the 7- isomer are revised. Latest shell-model calculations employing two different effective interactions reproduce the experimental findings and support the new spin and parity assignments.

High-spin states in 103,105Mo, 103Nb, and the νh11/2 alignment

NASA Astrophysics Data System (ADS)

Hua, H.; Wu, C. Y.; Cline, D.; Hayes, A. B.; Teng, R.; Clark, R. M.; Fallon, P.; Macchiavelli, A. O.; Vetter, K.

2002-06-01

High-spin states in neutron-rich nuclei 103,105Mo,103Nb have been studied using the 238U(α,f) fusion-fission reaction. The deexcitation γ rays were detected by Gammasphere in coincidence with the detection of both fission fragments by the Rochester 4π heavy-ion detector array, CHICO. The measured fission kinematics were used to deduce the masses and velocity vectors for both fission fragments. This allowed Doppler-shift corrections to be applied to the observed γ rays on an event-by-event basis and the origin of γ rays from either fission fragment to be established. With such advantages, the yrast sequences for these nuclei have been extended to the band crossing region. This band crossing is ascribed to the alignment of a pair of h11/2 neutrons, which is supported by the observed blocking effect for the νh11/2 band in 105Mo while there is no evidence for blocking in the alignment measured for either the νd5/2 band in 103Mo or the πg9/2 band in 103Nb. The observed upbend, rather than the sharp backbend seen in the Ru-Pd region, indicates a strong interaction between the ground-state and the aligned h11/2 bands.

The entangled triplet pair state in acene and heteroacene materials

PubMed Central

Yong, Chaw Keong; Musser, Andrew J.; Bayliss, Sam L.; Lukman, Steven; Tamura, Hiroyuki; Bubnova, Olga; Hallani, Rawad K.; Meneau, Aurélie; Resel, Roland; Maruyama, Munetaka; Hotta, Shu; Herz, Laura M.; Beljonne, David; Anthony, John E.; Clark, Jenny; Sirringhaus, Henning

2017-01-01

Entanglement of states is one of the most surprising and counter-intuitive consequences of quantum mechanics, with potent applications in cryptography and computing. In organic materials, one particularly significant manifestation is the spin-entangled triplet-pair state, which mediates the spin-conserving fission of one spin-0 singlet exciton into two spin-1 triplet excitons. Despite long theoretical and experimental exploration, the nature of the triplet-pair state and inter-triplet interactions have proved elusive. Here we use a range of organic semiconductors that undergo singlet exciton fission to reveal the photophysical properties of entangled triplet-pair states. We find that the triplet pair is bound with respect to free triplets with an energy that is largely material independent (∼30 meV). During its lifetime, the component triplets behave cooperatively as a singlet and emit light through a Herzberg–Teller-type mechanism, resulting in vibronically structured photoluminescence. In photovoltaic blends, charge transfer can occur from the bound triplet pairs with >100% photon-to-charge conversion efficiency. PMID:28699637

The entangled triplet pair state in acene and heteroacene materials

NASA Astrophysics Data System (ADS)

Yong, Chaw Keong; Musser, Andrew J.; Bayliss, Sam L.; Lukman, Steven; Tamura, Hiroyuki; Bubnova, Olga; Hallani, Rawad K.; Meneau, Aurélie; Resel, Roland; Maruyama, Munetaka; Hotta, Shu; Herz, Laura M.; Beljonne, David; Anthony, John E.; Clark, Jenny; Sirringhaus, Henning

2017-07-01

Entanglement of states is one of the most surprising and counter-intuitive consequences of quantum mechanics, with potent applications in cryptography and computing. In organic materials, one particularly significant manifestation is the spin-entangled triplet-pair state, which mediates the spin-conserving fission of one spin-0 singlet exciton into two spin-1 triplet excitons. Despite long theoretical and experimental exploration, the nature of the triplet-pair state and inter-triplet interactions have proved elusive. Here we use a range of organic semiconductors that undergo singlet exciton fission to reveal the photophysical properties of entangled triplet-pair states. We find that the triplet pair is bound with respect to free triplets with an energy that is largely material independent (~30 meV). During its lifetime, the component triplets behave cooperatively as a singlet and emit light through a Herzberg-Teller-type mechanism, resulting in vibronically structured photoluminescence. In photovoltaic blends, charge transfer can occur from the bound triplet pairs with >100% photon-to-charge conversion efficiency.

Competing decay modes of a high-spin isomer in the proton-unbound nucleus ¹⁵⁸Ta*

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carroll, R. J.; Page, R. D.; Joss, D. T.

2015-01-01

An isomeric state at high spin and excitation energy was recently observed in the proton-unbound nucleus 158Ta. This state was observed to decay by both α and γ decay modes. The large spin change required to decay via γ-ray emission incurs a lifetime long enough for α decay to compete. The α decay has an energy of 8644(11) keV, which is among the highest observed in the region, a partial half-life of 440(70) μs and changes the spin by 11ℏ. In this study, additional evidence supporting the assignment of this α decay to the high-spin isomer in 158Ta will bemore » presented.« less

Electromagnetic processes in nucleus-nucleus collisions relating to space radiation research

NASA Technical Reports Server (NTRS)

Norbury, John W.

1992-01-01

Most of the papers within this report deal with electromagnetic processes in nucleus-nucleus collisions which are of concern in the space radiation program. In particular, the removal of one and two nucleons via both electromagnetic and strong interaction processes has been extensively investigated. The theory of relativistic Coulomb fission has also been developed. Several papers on quark models also appear. Finally, note that the theoretical methods developed in this work have been directly applied to the task of radiation protection of astronauts. This has been done by parameterizing the theoretical formalism in such a fashion that it can be used in cosmic ray transport codes.

Effect of transverse vibrations of fissile nuclei on the angular and spin distributions of low-energy fission fragments

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bunakov, V. E.; Kadmensky, S. G., E-mail: kadmensky@phys.vsu.ru; Lyubashevsky, D. E.

2016-05-15

It is shown that A. Bohr’s classic theory of angular distributions of fragments originating from low-energy fission should be supplemented with quantum corrections based on the involvement of a superposition of a very large number of angular momenta L{sub m} in the description of the relative motion of fragments flying apart along the straight line coincidentwith the symmetry axis. It is revealed that quantum zero-point wriggling-type vibrations of the fissile system in the vicinity of its scission point are a source of these angular momenta and of high fragment spins observed experimentally.

Possibility of synthesizing a doubly magic superheavy nucleus

NASA Astrophysics Data System (ADS)

Aritomo, Y.

2007-02-01

The possibility of synthesizing a doubly magic superheavy nucleus, 298114184, is investigated on the basis of fluctuation-dissipation dynamics. In order to synthesize this nucleus, we must generate more neutron-rich compound nuclei because of the neutron emissions from excited compound nuclei. The compound nucleus 304114 has two advantages to achieving a high survival probability. First, because of low neutron separation energy and rapid cooling, the shell correction energy recovers quickly. Secondly, owing to neutron emissions, the neutron number in the nucleus approaches that of the double closed shell and the nucleus attains a large fission barrier. Because of these two effects, the survival probability of 304114 does not decrease until the excitation energy E*=50 MeV. These properties lead to a rather high evaporation residue cross section.

Photon-induced Fission Product Yield Measurements on 235U, 238U, and 239Pu

NASA Astrophysics Data System (ADS)

Krishichayan, Fnu; Bhike, M.; Tonchev, A. P.; Tornow, W.

2015-10-01

During the past three years, a TUNL-LANL-LLNL collaboration has provided data on the fission product yields (FPYs) from quasi-monoenergetic neutron-induced fission of 235U, 238U, and 239Pu at TUNL in the 0.5 to 15 MeV energy range. Recently, we have extended these experiments to photo-fission. We measured the yields of fission fragments ranging from 85Kr to 147Nd from the photo-fission of 235U, 238U, and 239Pu using 13-MeV mono-energetic photon beams at the HIGS facility at TUNL. First of its kind, this measurement will provide a unique platform to explore the effect of the incoming probe on the FPYs, i.e., photons vs. neutrons. A dual-fission ionization chamber was used to determine the number of fissions in the targets and these samples (along with Au monitor foils) were gamma-ray counted in the low-background counting facility at TUNL. Details of the experimental set-up and results will be presented and compared to the FPYs obtained from neutron-induced fission at the same excitation energy of the compound nucleus. Work supported in part by the NNSA-SSAA Grant No. DE-NA0001838.

The 4-dimensional Langevin approach to low energy nuclear fission

NASA Astrophysics Data System (ADS)

Ivanyuk, F. A.; Ishizuka, C.; Usang, M. D.; Chiba, S.

2018-03-01

We applied the four-dimensional Langevin approach to the description of fission of 235U by neutrons and calculated the dependence of the excitation energy of fission fragments on their mass number. For this we have fitted the compact just-before-scission configuration obtained by the Langevin calculations by the two separated fragments and calculated the intrinsic excitation and the deformation energy of each fragment accurately taking into account the shell and pairing effects and their dependence on the temperature and mass of the fragments. For the sharing of energy between the fission fragments we have used the simplest and most reliable assumption - the temperature of each fragment immediately after the neck rupture is the same as the temperature of mother nucleus just before scission. The calculated excitation energy of fission fragments clearly demonstrates the saw-tooth structure in the dependence on fragment mass number.

Near-barrier Fusion Evaporation and Fission of 28Si+174Yb and 32S+170Er

NASA Astrophysics Data System (ADS)

Wang, Dongxi; Lin, Chengjian; Jia, Huiming; Ma, Nanru; Sun, Lijie; Xu, Xinxing; Yang, Lei; Yang, Feng; Zhang, Huanqiao; Bao, Pengfei

2017-11-01

Fusion evaporation residues and fission fragments have been measured, respectively, at energies around the Coulomb barrier for the 28Si+174Yb and 32S+170Er systems forming the same compound nucleus 202Po. The excitation function of fusion evaporation, fission as well as capture reactions were deduced. Coupled-channels analyses reveal that couplings to the deformations of targets and the two-phonon states of projectiles contribute much to the enhancement of capture cross sections at sub-barrier energies. The mass and total kinetic energy of fission fragments were deduced by the time-difference method assuming full momentum transfer in a two-body kinematics. The mass-energy and mass-angle distributions were obtained and no obvious quasi-fission components were observed in this bombarding energy range. Further, mass distributions of fission fragments were fitted to extract their widths. Results show that the mass widths decrease monotonically with decreasing energy, but might start to increase when Ec.m./VB < 0.95 for both systems.

In-beam Fission Study at JAEA

NASA Astrophysics Data System (ADS)

Nishio, Katsuhisa

2013-12-01

Fission fragment mass distributions were measured in heavy-ion induced fissions using 238U target nucleus. The measured mass distributions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and quasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their incident energy dependence. Fusion probability was determined in the analysis. Evaporation residue cross sections were calculated with a statistical model in the reactions of 30Si + 238U and 34S + 238U using the obtained fusion probability in the entrance channel. The results agree with the measured cross sections for seaborgium and hassium isotopes.

In-beam fission study for Heavy Element Synthesis

NASA Astrophysics Data System (ADS)

Nishio, Katsuhisa

2013-12-01

Fission fragment mass distributions were measured in heavy-ion induced fissions using 238U target nucleus. The measured mass distributions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and qasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their incident energy dependence. Fusion probability was determined in the analysis. Evaporation residue cross sections were calculated with a statistical model in the reactions of 30Si + 238U and 34S + 238U using the obtained fusion probability in the entrance channel. The results agree with the measured cross sections for seaborgium and hassium isotopes.

Real causes of apparent abnormal results in heavy ion reactions

NASA Astrophysics Data System (ADS)

Mandaglio, G.; Nasirov, A. K.; Anastasi, A.; Curciarello, F.; De Leo, V.; Fazio, G.; Giardina, G.

2015-06-01

We study the effect of the static characteristics of nuclei and dynamics of the nucleus-nucleus interaction in the capture stage of reaction, in the competition between quasifission and complete fusion processes, as well as the angular momentum dependence of the competition between fission and evaporation processes along the de-excitation cascade of the compound nucleus. The results calculated for the mass-asymmetric and less mass-asymmetric reactions in the entrance channel are analyzed in order to investigate the role of the dynamical effects on the yields of the evaporation residue nuclei. We also discuss about uncertainties at the extraction of such relevant physical quantities as Γn/Γtot ratio or also excitation functions from the experimental results due to the not always realistic assumptions in the treatment and analysis of the detected events. This procedure can lead to large ambiguity when the complete fusion process is strongly hindered or when the fast fission contribution is large. We emphasize that a refined multiparameter model of the reaction dynamics as well as a more detailed and checked data analysis are strongly needed in heavy-ion collisions.

UCP2 regulates mitochondrial fission and ventromedial nucleus control of glucose responsiveness

PubMed Central

Toda, Chitoku; Kim, Jung Dae; Impellizzeri, Daniela; Cuzzocrea, Salvatore; Liu, Zhong-Wu; Diano, Sabrina

2016-01-01

Summary The ventromedial nucleus of the hypothalamus (VMH) plays a critical role in regulating systemic glucose homeostasis. How neurons in this brain area adapt to the changing metabolic environment to regulate circulating glucose levels is ill-defined. Here we show that glucose load results in mitochondrial fission and reduced reactive oxygen species in VMH neurons mediated by dynamin-related peptide 1 (DRP1) under the control of uncoupling protein 2 (UCP2). Probed by genetic manipulations and chemical-genetic control of VMH neuronal circuitry, we unmasked that this mitochondrial adaptation determines the size of the pool of glucose-excited neurons in the VMH, and, that this process regulates systemic glucose homoeostasis. Thus, our data unmasked a critical cellular biological process controlled by mitochondrial dynamics in VMH regulation of systemic glucose homeostasis. PMID:26919426

UCP2 Regulates Mitochondrial Fission and Ventromedial Nucleus Control of Glucose Responsiveness.

PubMed

Toda, Chitoku; Kim, Jung Dae; Impellizzeri, Daniela; Cuzzocrea, Salvatore; Liu, Zhong-Wu; Diano, Sabrina

2016-02-25

The ventromedial nucleus of the hypothalamus (VMH) plays a critical role in regulating systemic glucose homeostasis. How neurons in this brain area adapt to the changing metabolic environment to regulate circulating glucose levels is ill defined. Here, we show that glucose load results in mitochondrial fission and reduced reactive oxygen species in VMH neurons mediated by dynamin-related peptide 1 (DRP1) under the control of uncoupling protein 2 (UCP2). Probed by genetic manipulations and chemical-genetic control of VMH neuronal circuitry, we unmasked that this mitochondrial adaptation determines the size of the pool of glucose-excited neurons in the VMH and that this process regulates systemic glucose homeostasis. Thus, our data unmasked a critical cellular biological process controlled by mitochondrial dynamics in VMH regulation of systemic glucose homeostasis. Copyright © 2016 Elsevier Inc. All rights reserved.

A rapid decrease in the rotation rate of comet 41P/Tuttle–Giacobini–Kresák

NASA Astrophysics Data System (ADS)

Bodewits, Dennis; Farnham, Tony L.; Kelley, Michael S. P.; Knight, Matthew M.

2018-01-01

Cometary outgassing can produce torques that change the spin state of the cometary nucleus, which in turn influences the evolution and lifetime of the comet. If these torques increase the rate of rotation to the extent that centripetal forces exceed the material strength of the nucleus, the comet can fragment. Torques that slow down the rotation can cause the spin state to become unstable, but if the torques persist the nucleus can eventually reorient itself and the rotation rate can increase again. Simulations predict that most comets go through a short phase of rapid changes in spin state, after which changes occur gradually over longer times. Here we report observations of comet 41P/Tuttle–Giacobini–Kresák during its close approach to Earth (0.142 astronomical units, approximately 21 million kilometres, on 1 April 2017) that reveal a rapid decrease in rotation rate. Between March and May 2017, the apparent rotation period of the nucleus increased from 20 hours to more than 46 hours—a rate of change of more than an order of magnitude larger than has hitherto been measured. This phenomenon must have been caused by the gas emission from the comet aligning in such a way that it produced an anomalously strong torque that slowed the spin rate of the nucleus. The behaviour of comet 41P/Tuttle–Giacobini–Kresák suggests that it is in a distinct evolutionary state and that its rotation may be approaching the point of instability.

An Update on Binary Formation by Rotational Fission

NASA Astrophysics Data System (ADS)

Tohline, Joel E.; Durisen, Richard H.

During the 1980s, numerical simulations showed that dynamic growth of a barlike mode in initially axisymmetric, equilibrium protostars does not lead to prompt binary formation, i. e., fission. Instead, such evolutions usually produce a dynamically stable, spinning barlike configuration. In recent years, this result has been confirmed by numerous groups using a variety of different hydrodynamical tools, and stability analyses have convincingly shown that fission does not occur in such systems because gravitational torques cause nonlinear saturation of the mode amplitude. Other possible routes to fission have been much less well scrutinized because they rely upon a detailed understanding of the structure and stability of initially nonaxisymmetric structures and/or evolutions that are driven by secular, rather than dynamic processes. Efforts are underway to examine these other fission scenarios.

Single-level resonance parameters fit nuclear cross-sections

NASA Technical Reports Server (NTRS)

Drawbaugh, D. W.; Gibson, G.; Miller, M.; Page, S. L.

1970-01-01

Least squares analyses of experimental differential cross-section data for the U-235 nucleus have yielded single level Breit-Wigner resonance parameters that fit, simultaneously, three nuclear cross sections of capture, fission, and total.

Transfer-induced fission in inverse kinematics: Impact on experimental and evaluated nuclear data bases

NASA Astrophysics Data System (ADS)

Farget, F.; Caamaño, M.; Ramos, D.; Rodrıguez-Tajes, C.; Schmidt, K.-H.; Audouin, L.; Benlliure, J.; Casarejos, E.; Clément, E.; Cortina, D.; Delaune, O.; Derkx, X.; Dijon, A.; Doré, D.; Fernández-Domınguez, B.; Gaudefroy, L.; Golabek, C.; Heinz, A.; Jurado, B.; Lemasson, A.; Paradela, C.; Roger, T.; Salsac, M. D.; Schmitt, C.

2015-12-01

Inverse kinematics is a new tool to study nuclear fission. Its main advantage is the possibility to measure with an unmatched resolution the atomic number of fission fragments, leading to new observables in the properties of fission-fragment distributions. In addition to the resolution improvement, the study of fission based on nuclear collisions in inverse kinematics beneficiates from a larger view with respect to the neutron-induced fission, as in a single experiment the number of fissioning systems and the excitation energy range are widden. With the use of spectrometers, mass and kinetic-energy distributions may now be investigated as a function of the proton and neutron number sharing. The production of fissioning nuclei in transfer reactions allows studying the isotopic yields of fission fragments as a function of the excitation energy. The higher excitation energy resulting in the fusion reaction leading to the compound nucleus 250Cf at an excitation energy of 45MeV is also presented. With the use of inverse kinematics, the charge polarisation of fragments at scission is now revealed with high precision, and it is shown that it cannot be neglected, even at higher excitation energies. In addition, the kinematical properties of the fragments inform on the deformation configuration at scission.

Gamma rays as probe of fission and quasi-fission dynamics in the reaction 32S + 197Au near the Coulomb barrier

NASA Astrophysics Data System (ADS)

Pulcini, A.; Vardaci, E.; Kozulin, E.; Ashaduzzaman, M.; Borcea, C.; Bracco, A.; Brambilla, S.; Calinescu, S.; Camera, F.; Ciemala, M.; de Canditiis, B.; Dorvaux, O.; Harca, I. M.; Itkis, I.; Kirakosyan, V. V.; Knyazheva, G.; Kozulina, N.; Kolesov, I. V.; La Rana, G.; Maj, A.; Matea, I.; Novikov, K.; Petrone, C.; Quero, D.; Rath, P.; Saveleva, E.; Schmitt, C.; Sposito, G.; Stezowski, O.; Trzaska, W. H.; Wilson, J.

2018-05-01

Compound nucleus fission and quasi-fission are both binary decay channels whose common properties make the experimental separation between them difficult. A way to achieve this separation could be to probe the angular momentum of the binary fragments. This can be done detecting gamma rays in coincidence with the two fragments. As a case study, the reaction 32S + 197Au near the Coulomb barrier has been performed at the Tandem ALTO facility at IPN ORSAY. ORGAM and PARIS, two different gamma detectors arrays, are coupled with the CORSET detector, a two-arm time-of-flight spectrometer. TOF-TOF data were analyzed to reconstruct the mass-energy distribution of the primary fragments coupled with gamma multiplicity and spectroscopic analysis. Preliminary results of will be shown.

Staggering of angular momentum distribution in fission

NASA Astrophysics Data System (ADS)

Tamagno, Pierre; Litaize, Olivier

2018-03-01

We review here the role of angular momentum distributions in the fission process. To do so the algorithm implemented in the FIFRELIN code [?] is detailed with special emphasis on the place of fission fragment angular momenta. The usual Rayleigh distribution used for angular momentum distribution is presented and the related model derivation is recalled. Arguments are given to justify why this distribution should not hold for low excitation energy of the fission fragments. An alternative ad hoc expression taking into account low-lying collectiveness is presented as has been implemented in the FIFRELIN code. Yet on observables currently provided by the code, no dramatic impact has been found. To quantify the magnitude of the impact of the low-lying staggering in the angular momentum distribution, a textbook case is considered for the decay of the 144Ba nucleus with low excitation energy.

Clusterization in Ternary Fission

NASA Astrophysics Data System (ADS)

Kamanin, D. V.; Pyatkov, Y. V.

This lecture notes are devoted to the new kind of ternary decay of low excited heavy nuclei called by us "collinear cluster tri-partition" (CCT) due to the features of the effect observed, namely, decay partners fly away almost collinearly and at least one of them has magic nucleon composition. At the early stage of our work the process of "true ternary fission" (fission of the nucleus into three fragments of comparable masses) was considered to be undiscovered for low excited heavy nuclei. Another possible prototype—three body cluster radioactivity—was also unknown. The most close to the CCT phenomenon, at least cinematically, stands so called "polar emission", but only very light ions (up to isotopes of Be) were observed so far.

The Non-Adiabatic dynamics of Singlet Fission in Polyacenes

NASA Astrophysics Data System (ADS)

Bradforth, Stephen

2015-03-01

Singlet fission involves the splitting of a single excitation into two coupled triplet excitations and is manifested in an increasing range of aromatic crystals and amorphous thin films. If the energy of the lowest triplet state is one half (or less) of the first singlet excited state, as it is for tetracene or pentacene and their derivatives, singlet fission may occur between two adjacent chromophores. Since there is no change in the overall spin state of the system, singlet fission can be exceptionally fast, occuring on the fs - ps range. If the triplets can diffuse away from the fission site they are available for harvesting as a dissociated carriers with up to two charge carrier pairs per absorbed photon. The possibility of recovering excess energy above the material band gap (in this case determined by the triplet energy) when a higher energy photon is absorbed has led to great recent interest in exploiting this process for increased efficiency solar energy harvesting. The nature of the electronic couplings between the chromophores, intermediate electronic configurations, and the role of entropy in the spin-allowed primary fission event have all come under great scrutiny. Results from a series of femtosecond spectroscopy experiments on a variety of amorphous thin films, nanoparticles and isolated acene dimer compounds will be presented that shed light on the electronic intermediate states key to the efficiency and speed of this process. Work supported as part of the Center for Energy Nanoscience, an Energy Frontier Research Center funded by the U.S. Department of Energy (DE-SC0001013).

α versus non-α cluster decays of the excited compound nucleus *124Ce using various formulations of the nuclear proximity potential

NASA Astrophysics Data System (ADS)

Kaur, Arshdeep; Chopra, Sahila; Gupta, Raj K.

2015-06-01

The earlier study of *124Ce formed in the 32S+92Mo reaction at an above barrier beam energy of 150 MeV, using the pocket formula of Blocki et al. for the nuclear proximity potential in the dynamical cluster-decay model (DCM), is extended to the use of other nuclear interaction potentials derived from the Skyrme energy density functional (SEDF) based on the semiclassical extended Thomas Fermi (ETF) approach under the frozen density approximation. The Skyrme forces used are the old SII, SIII, SIV, SKa, SkM, and SLy4 and new GSkI and KDE0(v1), given for both normal and isospin-rich nuclei. It is found that the α -nucleus structure, over the non-α nucleus structure, is preferred for only two Skyrme forces, the SIII and KDE0(v1). An extended intermediate mass fragments (IMFs) window, along with the new decay region of heavy mass fragments (HMFs) and the near-symmetric and symmetric fission fragments which, on adding the complementary heavy fragments, corresponds to (A /2 )±12 mass region of the fusion-fission (ff) process, are predicted by considering cross sections of orders observed in the experiment under study. For the predicted (total) fusion cross section, the survival probability Psurv of the compound nucleus (CN) against fission is shown to be very small because of the very large predicted ff component. On the other hand, the CN formation probability PCN is found to be nearly equal to 1, and hence the decay under study is a pure CN decay for all the nuclear potentials considered, since the estimated noncompound nucleus (nCN) content is almost negligible. We have also applied the extended-Wong model of Gupta and collaborators, and find that the ℓmax values and total fusion cross sections are of the same order as for the DCM. Thus, the extended-Wong model, which describes only the total fusion cross section in terms of the barrier characteristics of the entrance channel nuclei, could be useful for initial experimental studies to be fully treated using the DCM for all the observed decay products.

Anisotropy of the angular distribution of fission fragments in heavy-ion fusion-fission reactions: The influence of the level-density parameter and the neck thickness

NASA Astrophysics Data System (ADS)

Naderi, D.; Pahlavani, M. R.; Alavi, S. A.

2013-05-01

Using the Langevin dynamical approach, the neutron multiplicity and the anisotropy of angular distribution of fission fragments in heavy ion fusion-fission reactions were calculated. We applied one- and two-dimensional Langevin equations to study the decay of a hot excited compound nucleus. The influence of the level-density parameter on neutron multiplicity and anisotropy of angular distribution of fission fragments was investigated. We used the level-density parameter based on the liquid drop model with two different values of the Bartel approach and Pomorska approach. Our calculations show that the anisotropy and neutron multiplicity are affected by level-density parameter and neck thickness. The calculations were performed on the 16O+208Pb and 20Ne+209Bi reactions. Obtained results in the case of the two-dimensional Langevin with a level-density parameter based on Bartel and co-workers approach are in better agreement with experimental data.

Unified model for singlet fission within a non-conjugated covalent pentacene dimer

NASA Astrophysics Data System (ADS)

Basel, Bettina S.; Zirzlmeier, Johannes; Hetzer, Constantin; Phelan, Brian T.; Krzyaniak, Matthew D.; Reddy, S. Rajagopala; Coto, Pedro B.; Horwitz, Noah E.; Young, Ryan M.; White, Fraser J.; Hampel, Frank; Clark, Timothy; Thoss, Michael; Tykwinski, Rik R.; Wasielewski, Michael R.; Guldi, Dirk M.

2017-05-01

When molecular dimers, crystalline films or molecular aggregates absorb a photon to produce a singlet exciton, spin-allowed singlet fission may produce two triplet excitons that can be used to generate two electron-hole pairs, leading to a predicted ~50% enhancement in maximum solar cell performance. The singlet fission mechanism is still not well understood. Here we report on the use of time-resolved optical and electron paramagnetic resonance spectroscopy to probe singlet fission in a pentacene dimer linked by a non-conjugated spacer. We observe the key intermediates in the singlet fission process, including the formation and decay of a quintet state that precedes formation of the pentacene triplet excitons. Using these combined data, we develop a single kinetic model that describes the data over seven temporal orders of magnitude both at room and cryogenic temperatures.

Unified model for singlet fission within a non-conjugated covalent pentacene dimer.

PubMed

Basel, Bettina S; Zirzlmeier, Johannes; Hetzer, Constantin; Phelan, Brian T; Krzyaniak, Matthew D; Reddy, S Rajagopala; Coto, Pedro B; Horwitz, Noah E; Young, Ryan M; White, Fraser J; Hampel, Frank; Clark, Timothy; Thoss, Michael; Tykwinski, Rik R; Wasielewski, Michael R; Guldi, Dirk M

2017-05-18

When molecular dimers, crystalline films or molecular aggregates absorb a photon to produce a singlet exciton, spin-allowed singlet fission may produce two triplet excitons that can be used to generate two electron-hole pairs, leading to a predicted ∼50% enhancement in maximum solar cell performance. The singlet fission mechanism is still not well understood. Here we report on the use of time-resolved optical and electron paramagnetic resonance spectroscopy to probe singlet fission in a pentacene dimer linked by a non-conjugated spacer. We observe the key intermediates in the singlet fission process, including the formation and decay of a quintet state that precedes formation of the pentacene triplet excitons. Using these combined data, we develop a single kinetic model that describes the data over seven temporal orders of magnitude both at room and cryogenic temperatures.

Radionuclide Basics: Tritium

EPA Pesticide Factsheets

Tritium is a hydrogen atom that has two neutrons in the nucleus and one proton. It is radioactive and behaves like other forms of hydrogen in the environment. Tritium is produced naturally in the upper atmosphere and as a byproduct of nuclear fission.

The entrance channel effects on the deexcitation ways of the same compound nucleus at a fixed excitation energy

NASA Astrophysics Data System (ADS)

Anastasi, A.; Mandaglio, G.; Curciarello, F.; Nasirov, A. K.; Fazio, G.; Giardina, G.

2018-05-01

The investigation of various properties of deexcitation of the same 220Th compound nucleus (CN), formed by the different mass (charge) asymmetric 16O+204Pb, 40Ar+180Hf, 82Se+138Ba and 96Zr+124Sn reactions is presented. The effective fission barrier < B fis > value, as a function of the excitation energy {E}CN* , determined for each intermediate excited nucleus reached along the deexcitation cascade of the CN obtained by the four considered reactions is strongly sensitive to the various orbital angular momentum L=ℓℏ distributions of CN formed with the same excitation energy {E}CN* by the various entrance channels. Therefore, the competition between the fission and evaporation of light particles (neutron, proton, and α-particle) processes along the deexcitation cascade of CN is dependent on the orbital angular momentum distribution of CN. In fact, the ratio between the evaporation residue cross sections obtained when also the charged particles are emitted and the ones obtained after neutron emission only for the same CN with a fixed excitation energy {E}CN* is sensitive to the mass (charge) asymmetry of the entrance channel.

Microscopic Phase-Space Exploration Modeling of ^{258}Fm Spontaneous Fission.

PubMed

Tanimura, Yusuke; Lacroix, Denis; Ayik, Sakir

2017-04-14

We show that the total kinetic energy (TKE) of nuclei after the spontaneous fission of ^{258}Fm can be well reproduced using simple assumptions on the quantum collective phase space explored by the nucleus after passing the fission barrier. Assuming energy conservation and phase-space exploration according to the stochastic mean-field approach, a set of initial densities is generated. Each density is then evolved in time using the nuclear time-dependent density-functional theory with pairing. This approach goes beyond the mean-field theory by allowing spontaneous symmetry breaking as well as a wider dynamical phase-space exploration leading to larger fluctuations in collective space. The total kinetic energy and mass distributions are calculated. New information on the fission process: fluctuations in scission time, strong correlation between TKE and collective deformation, as well as prescission particle emission, are obtained. We conclude that fluctuations of the TKE and mass are triggered by quantum fluctuations.

High resolution gamma-ray spectroscopy and the fascinating angular momentum realm of the atomic nucleus

NASA Astrophysics Data System (ADS)

Riley, M. A.; Simpson, J.; Paul, E. S.

2016-12-01

In 1974 Aage Bohr and Ben Mottelson predicted the different ‘phases’ that may be expected in deformed nuclei as a function of increasing angular momentum and excitation energy all the way up to the fission limit. While admitting their picture was highly conjectural they confidently stated ‘...with the ingenious experimental approaches that are being developed, we may look forward with excitement to the detailed spectroscopic studies that will illuminate the behaviour of the spinning quantised nucleus’. High resolution gamma-ray spectroscopy has indeed been a major tool in studying the structure of atomic nuclei and has witnessed numerous significant advances over the last four decades. This article will select highlights from investigations at the Niels Bohr Institute, Denmark, and Daresbury Laboratory, UK, in the late 1970s and early 1980s, some of which have continued at other national laboratories in Europe and the USA to the present day. These studies illustrate the remarkable diversity of phenomena and symmetries exhibited by nuclei in the angular momentum-excitation energy plane that continue to surprise and fascinate scientists.

Nonaxial hexadecapole deformation effects on the fission barrier

NASA Astrophysics Data System (ADS)

Kardan, A.; Nejati, S.

2016-06-01

Fission barrier of the heavy nucleus 250Cf is analyzed in a multi-dimensional deformation space. This space includes two quadrupole (ɛ2,γ) and three hexadecapole deformation (ɛ40,ɛ42,ɛ44) parameters. The analysis is performed within an unpaired macroscopic-microscopic approach. Special attention is given to the effects of the axial and non-axial hexadecapole deformation shapes. It is found that the inclusion of the nonaxial hexadecapole shapes does not change the fission barrier heights, so it should be sufficient to minimize the energy in only one degree of freedom in the hexadecapole space ɛ4. The role of hexadecapole deformation parameters is also discussed on the Lublin-Strasbourg drop (LSD) macroscopic and the Strutinsky shell energies.

Mass and angular distributions of the reaction products in heavy ion collisions

NASA Astrophysics Data System (ADS)

Nasirov, A. K.; Giardina, G.; Mandaglio, G.; Kayumov, B. M.; Tashkhodjaev, R. B.

2018-05-01

The optimal reactions and beam energies leading to synthesize superheavy elements is searched by studying mass and angular distributions of fission-like products in heavy-ion collisions since the evaporation residue cross section consists an ignorable small part of the fusion cross section. The intensity of the yield of fission-like products allows us to estimate the probability of the complete fusion of the interacting nuclei. The overlap of the mass and angular distributions of the fusion-fission and quasifission products causes difficulty at estimation of the correct value of the probability of the compound nucleus formation. A study of the mass and angular distributions of the reaction products is suitable key to understand the interaction mechanism of heavy ion collisions.

First-Principle Characterization for Singlet Fission Couplings.

PubMed

Yang, Chou-Hsun; Hsu, Chao-Ping

2015-05-21

The electronic coupling for singlet fission, an important parameter for determining the rate, has been found to be too small unless charge-transfer (CT) components were introduced in the diabatic states, mostly through perturbation or a model Hamiltonian. In the present work, the fragment spin difference (FSD) scheme was generalized to calculate the singlet fission coupling. The largest coupling strength obtained was 14.8 meV for two pentacenes in a crystal structure, or 33.7 meV for a transition-state structure, which yielded a singlet fission lifetime of 239 or 37 fs, generally consistent with experimental results (80 fs). Test results with other polyacene molecules are similar. We found that the charge on one fragment in the S1 diabatic state correlates well with FSD coupling, indicating the importance of the CT component. The FSD approach is a useful first-principle method for singlet fission coupling, without the need to include the CT component explicitly.

Femtosecond stimulated Raman evidence for charge-transfer character in pentacene singlet fission.

PubMed

Hart, Stephanie M; Silva, W Ruchira; Frontiera, Renee R

2018-02-07

Singlet fission is a spin-allowed process in which an excited singlet state evolves into two triplet states. We use femtosecond stimulated Raman spectroscopy, an ultrafast vibrational technique, to follow the molecular structural evolution during singlet fission in order to determine the mechanism of this process. In crystalline pentacene, we observe the formation of an intermediate characterized by pairs of excited state peaks that are red- and blue-shifted relative to the ground state features. We hypothesize that these features arise from the formation of cationic and anionic species due to partial transfer of electron density from one pentacene molecule to a neighboring molecule. These observations provide experimental evidence for the role of states with significant charge-transfer character which facilitate the singlet fission process in pentacene. Our work both provides new insight into the singlet fission mechanism in pentacene and demonstrates the utility of structurally-sensitive time-resolved spectroscopic techniques in monitoring ultrafast processes.

Unified model for singlet fission within a non-conjugated covalent pentacene dimer

DOE PAGES

Basel, Bettina S.; Zirzlmeier, Johannes; Hetzer, Constantin; ...

2017-05-18

When molecular dimers, crystalline films or molecular aggregates absorb a photon to produce a singlet exciton, spin-allowed singlet fission may produce two triplet excitons that can be used to generate two electron–hole pairs, leading to a predicted B50% enhancement in maximum solar cell performance. The singlet fission mechanism is still not well understood. Here we report on the use of time-resolved optical and electron paramagnetic resonance spectroscopy to probe singlet fission in a pentacene dimer linked by a non-conjugated spacer. We observe the key intermediates in the singlet fission process, including the formation and decay of a quintet state thatmore » precedes formation of the pentacene triplet excitons. In conclusion, using these combined data, we develop a single kinetic model that describes the data over seven temporal orders of magnitude both at room and cryogenic temperatures.« less

Unified model for singlet fission within a non-conjugated covalent pentacene dimer

PubMed Central

Basel, Bettina S.; Zirzlmeier, Johannes; Hetzer, Constantin; Phelan, Brian T.; Krzyaniak, Matthew D.; Reddy, S. Rajagopala; Coto, Pedro B.; Horwitz, Noah E.; Young, Ryan M.; White, Fraser J.; Hampel, Frank; Clark, Timothy; Thoss, Michael; Tykwinski, Rik R.; Wasielewski, Michael R.; Guldi, Dirk M.

2017-01-01

When molecular dimers, crystalline films or molecular aggregates absorb a photon to produce a singlet exciton, spin-allowed singlet fission may produce two triplet excitons that can be used to generate two electron–hole pairs, leading to a predicted ∼50% enhancement in maximum solar cell performance. The singlet fission mechanism is still not well understood. Here we report on the use of time-resolved optical and electron paramagnetic resonance spectroscopy to probe singlet fission in a pentacene dimer linked by a non-conjugated spacer. We observe the key intermediates in the singlet fission process, including the formation and decay of a quintet state that precedes formation of the pentacene triplet excitons. Using these combined data, we develop a single kinetic model that describes the data over seven temporal orders of magnitude both at room and cryogenic temperatures. PMID:28516916

Thermodynamics of fission products in UO(2 ± x).

PubMed

Nerikar, P V; Liu, X-Y; Uberuaga, B P; Stanek, C R; Phillpot, S R; Sinnott, S B

2009-10-28

The stabilities of selected fission products-Xe, Cs, and Sr-are investigated as a function of non-stoichiometry x in UO(2 ± x). In particular, density functional theory (DFT) is used to calculate the incorporation and solution energies of these fission products at the anion and cation vacancy sites, at the divacancy, and at the bound Schottky defect. In order to reproduce the correct insulating state of UO(2), the DFT calculations are performed using spin polarization and with the Hubbard U term. In general, higher charge defects are more soluble in the fuel matrix and the solubility of fission products increases as the hyperstoichiometry increases. The solubility of fission product oxides is also explored. Cs(2)O is observed as a second stable phase and SrO is found to be soluble in the UO(2) matrix for all stoichiometries. These observations mirror experimentally observed phenomena.

Vibronically coherent ultrafast triplet-pair formation and subsequent thermally activated dissociation control efficient endothermic singlet fission

NASA Astrophysics Data System (ADS)

Stern, Hannah L.; Cheminal, Alexandre; Yost, Shane R.; Broch, Katharina; Bayliss, Sam L.; Chen, Kai; Tabachnyk, Maxim; Thorley, Karl; Greenham, Neil; Hodgkiss, Justin M.; Anthony, John; Head-Gordon, Martin; Musser, Andrew J.; Rao, Akshay; Friend, Richard H.

2017-12-01

Singlet exciton fission (SF), the conversion of one spin-singlet exciton (S1) into two spin-triplet excitons (T1), could provide a means to overcome the Shockley-Queisser limit in photovoltaics. SF as measured by the decay of S1 has been shown to occur efficiently and independently of temperature, even when the energy of S1 is as much as 200 meV less than that of 2T1. Here we study films of triisopropylsilyltetracene using transient optical spectroscopy and show that the triplet pair state (TT), which has been proposed to mediate singlet fission, forms on ultrafast timescales (in 300 fs) and that its formation is mediated by the strong coupling of electronic and vibrational degrees of freedom. This is followed by a slower loss of singlet character as the excitation evolves to become only TT. We observe the TT to be thermally dissociated on 10-100 ns timescales to form free triplets. This provides a model for 'temperature-independent' efficient TT formation and thermally activated TT separation.

Maruhn-Greiner Maximum of Uranium Fission for Confirmation of Low Energy Nuclear Reactions LENR via a Compound Nucleus with Double Magic Numbers

NASA Astrophysics Data System (ADS)

Hora, H.; Miley, G. H.

2007-12-01

One of the most convincing facts about LENR due to deuterons of very high concentration in host metals as palladium is the measurement of the large scale minimum of the reaction probability depending on the nucleon number A of generated elements at A = 153 where a local maximum was measured. This is similar to the fission of uranium at A = 119 where the local maximum follows from the Maruhn-Greiner theory if the splitting nuclei are excited to about MeV energy. The LENR generated elements can be documented any time after the reaction by SIMS or K-shell X-ray excitation to show the very unique distribution with the local maximum. An explanation is based on the strong Debye screening of the Maxwellian deuterons within the degenerate rigid electron background especially within the swimming electron layer at the metal surface or at interfaces. The deuterons behave like neutrals at distances of about 2 picometers. They may form clusters due to soft attraction in the range above thermal energy. Clusters of 10 pm diameter may react over long time probabilities (megaseconds) with Pd nuclei leading to a double magic number compound nucleus which splits like in fission to the A = 153 element distribution.

Persistence of collective behavior at high spin in the N = 88 nucleus Tb 153

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hartley, D. J.; Riley, M. A.; Wang, X.

Excited states in the N = 88 nucleus Tb-153 were observed up to spin similar to 40 in an experiment utilizing the Gammasphere array. The Tb-153 states were populated in a weak alpha 4n evaporation channel of the Cl-37 + Sn-124 reaction. Two previously known sequences were extended to higher spins, and a new decoupled structure was identified. The pi h(11/2) band was observed in the spin region where other N = 88 isotopes exhibit effects of prolate to oblate shape changes leading to band termination along the yrast line, whereas Tb-153 displays a persistent collective behavior. However, minor perturbationsmore » of the very highest state in both signatures of this h(11/2) band are observed, which perhaps signal the start of the transition towards band termination.« less

Organic semiconductors: Dynamic duos

NASA Astrophysics Data System (ADS)

Wasielewski, Michael R.

2017-02-01

The discovery of intermediate high-spin multiexciton states with surprisingly long lifetimes provides new opportunities for engineering singlet fission, which may also provide an intriguing route to quantum information and spintronic applications.

Effects of molecular packing in organic crystals on singlet fission with ab initio many body perturbation theory

NASA Astrophysics Data System (ADS)

Haber, Jonah; Refaely-Abramson, Sivan; da Jornada, Felipe H.; Louie, Steven G.; Neaton, Jeffrey B.

Multi-exciton generation processes, in which multiple charge carriers are generated from a single photon, are mechanisms of significant interest for achieving efficiencies beyond the Shockley-Queisser limit of conventional p-n junction solar cells. One well-studied multiexciton process is singlet fission, whereby a singlet decays into two spin-correlated triplet excitons. Here, we use a newly developed computational approach to calculate singlet-fission coupling terms and rates with an ab initio Green's function formalism based on many-body perturbation theory (MBPT) within the GW approximation and the Bethe-Salpeter equation approach. We compare results for crystalline pentacene and TIPS-pentacene and explore the effect of molecular packing on the singlet fission mechanism. This work is supported by the Department of Energy.

Spontaneous Fission Barriers Based on a Generalized Liquid Drop Model

NASA Astrophysics Data System (ADS)

Guo, Shu-Qing; Bao, Xiao-Jun; Li, Jun-Qing; Zhang, Hong-Fei

2014-05-01

The barrier against the spontaneous fission has been determined within the Generalized Liquid Drop Model (GLDM) including the mass and charge asymmetry, and the proximity energy. The shell correction of the spherical parent nucleus is calculated by using the Strutinsky method, and the empirical shape-dependent shell correction is employed during the deformation process. A quasi-molecular shape sequence has been defined to describe the whole process from one-body shape to two-body shape system, and a two-touching-ellipsoid is adopted when the superdeformed one-body system reaches the rupture point. On these bases the spontaneous fission barriers are systematically studied for nuclei from 230Th to 249Cm for different possible exiting channels with the different mass and charge asymmetries. The double, and triple bumps are found in the fission potential energy in this region, which roughly agree with the experimental results. It is found that at around Sn-like fragment the outer fission barriers are lower, while the partner of the Sn-like fragment is in the range near 108Ru where the ground-state mass is lowered by allowing axially symmetric shapes. The preferable fission channels are distinctly pronounced, which should be corresponding to the fragment mass distributions.

Influence of the bud neck on nuclear envelope fission in Saccharomyces cerevisiae.

PubMed

Melloy, Patricia G; Rose, Mark D

2017-09-15

Studies have shown that nuclear envelope fission (karyokinesis) in budding yeast depends on cytokinesis, but not distinguished whether this was a direct requirement, indirect, because of cell cycle arrest, or due to bud neck-localized proteins impacting both processes. To determine the requirements for karyokinesis, we examined mutants conditionally defective for bud emergence and/or nuclear migration. The common mutant phenotype was completion of the nuclear division cycle within the mother cell, but karyokinesis did not occur. In the cdc24 swe1 mutant, at the non-permissive temperature, multiple nuclei accumulated within the unbudded cell, with connected nuclear envelopes. Upon return to the permissive temperature, the cdc24 swe1 mutant initiated bud emergence, but only the nucleus spanning the neck underwent fission suggesting that the bud neck region is important for fission initiation. The neck may be critical for either mechanical reasons, as the contractile ring might facilitate fission, or for regulatory reasons, as the site of a protein network regulating nuclear envelope fission, mitotic exit, and cytokinesis. We also found that 77-85% of pairs of septin mutant nuclei completed nuclear envelope fission. In addition, 27% of myo1Δ mutant nuclei completed karyokinesis. These data suggested that fission is not dependent on mechanical contraction at the bud neck, but was instead controlled by regulatory proteins there. Copyright © 2017 Elsevier Inc. All rights reserved.

Strongly exchange-coupled triplet pairs in an organic semiconductor

NASA Astrophysics Data System (ADS)

Weiss, Leah R.; Bayliss, Sam L.; Kraffert, Felix; Thorley, Karl J.; Anthony, John E.; Bittl, Robert; Friend, Richard H.; Rao, Akshay; Greenham, Neil C.; Behrends, Jan

2017-02-01

From biological complexes to devices based on organic semiconductors, spin interactions play a key role in the function of molecular systems. For instance, triplet-pair reactions impact operation of organic light-emitting diodes as well as photovoltaic devices. Conventional models for triplet pairs assume they interact only weakly. Here, using electron spin resonance, we observe long-lived, strongly interacting triplet pairs in an organic semiconductor, generated via singlet fission. Using coherent spin manipulation of these two-triplet states, we identify exchange-coupled (spin-2) quintet complexes coexisting with weakly coupled (spin-1) triplets. We measure strongly coupled pairs with a lifetime approaching 3 μs and a spin coherence time approaching 1 μs, at 10 K. Our results pave the way for the utilization of high-spin systems in organic semiconductors.

Evaporation channel as a tool to study fission dynamics

NASA Astrophysics Data System (ADS)

Di Nitto, A.; Vardaci, E.; La Rana, G.; Nadtochy, P. N.; Prete, G.

2018-03-01

The dynamics of the fission process is expected to affect the evaporation residue cross section because of the fission hindrance due to the nuclear viscosity. Systems of intermediate fissility constitute a suitable environment for testing such hypothesis since they are characterized by evaporation residue cross sections comparable or larger than the fission ones. Observables related to emitted charged particles, due to their relatively high emission probability, can be used to put stringent constraints on models describing the excited nucleus decay and to recognize the effects of fission dynamics. In this work model simulations are compared with the experimental data collected via the 32S +100 Mo reaction at Elab = 200 MeV. Consequently we pointed out, exploring an extended set of evaporation channel observables, the limits of the statistical model and the large improvement obtained with a dynamical model. Moreover we stress the importance of using an apparatus covering a large fraction of 4π to extract observables. Finally, we discuss the opportunity to measure more sensitive observables by a new detection device in operation at LNL.

Lipid droplets form from distinct regions of the cell in the fission yeast Schizosaccharomyces pombe

DOE Office of Scientific and Technical Information (OSTI.GOV)

Meyers, Alex; del Rio, Zuania P.; Beaver, Rachael A.

Eukaryotic cells store cholesterol/sterol esters (SEs) and triacylglycerols (TAGs) in lipid droplets, which form from the contiguous endoplasmic reticulum (ER) network. However, it is not known if droplets preferentially form from certain regions of the ER over others. Here, we used fission yeast Schizosaccharomyces pombe cells where the nuclear and cortical/peripheral ER domains are distinguishable by light microscopy to show that SE-enriched lipid droplets form away from the nucleus at the cell tips, whereas TAG-enriched lipid droplets form around the nucleus. Sterols localize to the regions of the cells where droplets enriched in SEs are observed. TAG droplet formation aroundmore » the nucleus appears to be a strong function of diacylglycerol (DAG) homeostasis with Cpt1p, which coverts DAG into phosphatidylcholine and phosphatidylethanolamine localized exclusively to the nuclear ER. Also, Dgk1p, which converts DAG into phosphatidic acid localized strongly to the nuclear ER over the cortical/peripheral ER. We also show that TAG more readily translocates from the ER to lipid droplets than do SEs. Lastly, the results augment the standard lipid droplet formation model, which has SEs and TAGs flowing into the same nascent lipid droplet regardless of its biogenesis point in the cell.« less

Lipid droplets form from distinct regions of the cell in the fission yeast Schizosaccharomyces pombe

DOE PAGES

Meyers, Alex; del Rio, Zuania P.; Beaver, Rachael A.; ...

2016-04-29

Eukaryotic cells store cholesterol/sterol esters (SEs) and triacylglycerols (TAGs) in lipid droplets, which form from the contiguous endoplasmic reticulum (ER) network. However, it is not known if droplets preferentially form from certain regions of the ER over others. Here, we used fission yeast Schizosaccharomyces pombe cells where the nuclear and cortical/peripheral ER domains are distinguishable by light microscopy to show that SE-enriched lipid droplets form away from the nucleus at the cell tips, whereas TAG-enriched lipid droplets form around the nucleus. Sterols localize to the regions of the cells where droplets enriched in SEs are observed. TAG droplet formation aroundmore » the nucleus appears to be a strong function of diacylglycerol (DAG) homeostasis with Cpt1p, which coverts DAG into phosphatidylcholine and phosphatidylethanolamine localized exclusively to the nuclear ER. Also, Dgk1p, which converts DAG into phosphatidic acid localized strongly to the nuclear ER over the cortical/peripheral ER. We also show that TAG more readily translocates from the ER to lipid droplets than do SEs. Lastly, the results augment the standard lipid droplet formation model, which has SEs and TAGs flowing into the same nascent lipid droplet regardless of its biogenesis point in the cell.« less

Shape coexistence in the N = 19 neutron-rich nucleus 31Mg explored by β-γ spectroscopy of spin-polarized 31Na

NASA Astrophysics Data System (ADS)

Nishibata, H.; Shimoda, T.; Odahara, A.; Morimoto, S.; Kanaya, S.; Yagi, A.; Kanaoka, H.; Pearson, M. R.; Levy, C. D. P.; Kimura, M.

2017-04-01

The structure of excited states in the neutron-rich nucleus 31Mg, which is in the region of the ;island of inversion; associated with the neutron magic number N = 20, is studied by β-γ spectroscopy of spin-polarized 31Na. Among the 31Mg levels below the one neutron separation energy of 2.3 MeV, the spin values of all five positive-parity levels are unambiguously determined by observing the anisotropic β decay. Two rotational bands with Kπ = 1 /2+ and 1 /2- are proposed based on the spins and energies of the levels. Comparison on a level-by-level basis is performed between the experimental results and theoretical calculations by the antisymmetrized molecular dynamics (AMD) plus generator coordinate method (GCM). It is found that various nuclear structures coexist in the low excitation energy region in 31Mg.

Prompt neutron emission and energy balance in 235U(n,f)

NASA Astrophysics Data System (ADS)

Göök, Alf; Hambsch, Franz-Josef; Oberstedt, Stephan

2017-09-01

Investigations of prompt fission neutron (PFN) emission are of importance in understanding the fission process in general and the sharing of excitation energy among the fission fragments in particular. Experimental activities at JRC-Geel on PFN emission in response to OECD/NEA nuclear data requests is presented in this contribution. The focus lies on on-going investigations of PFN emission from the reaction 235U(n,f) in the region of the resolved resonances taking place at the GELINA facility. For this reaction strong fluctuations of fission fragment mass distributions and mean total kinetic energy have been observed as a function of incident neutron energy in the resonance region. In addition, fluctuations of prompt neutron multiplicities have also been observed. The goal of the present study is to verify the current knowledge of PFN multiplicity fluctuations and to study correlations with fission fragment properties. The experiment employs a scintillation detector array for neutron detection, while fission fragment properties are determined via the double kinetic energy technique using a position sensitive twin ionization chamber. Results on PFN multiplicity correlations with fission fragment properties from the present study show significant differences compared to earlier studies on this reaction, induced by thermal neutrons. Specifically, the total kinetic energy dependence of the neutron multiplicity per fission shows an inverse slope FX1TKE/FX2ν approximately 35% weaker than observed in earlier studies of thermal neutron induced fission on 235U. The inverse slope is related to the energy carried away per emitted neutron and is, thereby, closely connected to the energy balance of the fission reaction. The present result should have strong impact on the modeling of both prompt neutron and prompt γ-ray emission in fission of the 236U compound nucleus.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Basel, Bettina S.; Zirzlmeier, Johannes; Hetzer, Constantin

When molecular dimers, crystalline films or molecular aggregates absorb a photon to produce a singlet exciton, spin-allowed singlet fission may produce two triplet excitons that can be used to generate two electron–hole pairs, leading to a predicted B50% enhancement in maximum solar cell performance. The singlet fission mechanism is still not well understood. Here we report on the use of time-resolved optical and electron paramagnetic resonance spectroscopy to probe singlet fission in a pentacene dimer linked by a non-conjugated spacer. We observe the key intermediates in the singlet fission process, including the formation and decay of a quintet state thatmore » precedes formation of the pentacene triplet excitons. In conclusion, using these combined data, we develop a single kinetic model that describes the data over seven temporal orders of magnitude both at room and cryogenic temperatures.« less

Investigation of High-Spin States in ^203Rn

NASA Astrophysics Data System (ADS)

Beausang, C. W.; Novak, J. R.; Caprio, M.; Casten, R. F.; Cederkall, J.; Cooper, J. R.; Krücken, R.; Wang, Z.; Zamfir, N. V.; Barton, C. J.

1999-10-01

High-spin states in ^203Rn were populated following the reaction ^34S + ^174Yb + 5n at beam energies ranging from 160 to 170 MeV. Gamma-rays were detected using the multi-Ge detector array YRAST Ball located at the Wright Nuclear Structure Laboratory. In addition the SCARY array, an array of 28 solar cell detectors, each 1 cm by 1 cm, was arranged around the target at backward angles. These were used to detect fission fragments and hence discriminate against the very large fission background encountered in this reaction. Following our excitation function measurement several transitions can be assigned to ^203Rn, where previously no information was available on excited states. Data analysis is continuing and preliminary results will be presented. This work is supported by the US-DOE under grant number DE-FG02-91ER-40609.

MODE OF FISSION OF BENZENE NUCLEUS IN THE MICRO-ORGANISMS AND REGULATION OF CELL GROWTH AND DIVISION BY BENZENE DERIVATIVES.

DTIC Science & Technology

as an amino donor in this microbial system. The conversion D-tryptophan to L-tryptophan in a cell-free system can be demonstrated when an electron acceptor, such as phenazine methosulfate, is present. (Author)

Measurement of the ROT effect in the neutron induced fission of 235U in the 0.3 eV resonance at a hot source of polarized neutrons

NASA Astrophysics Data System (ADS)

Kopatch, Yuri; Novitsky, Vadim; Ahmadov, Gadir; Gagarsky, Alexei; Berikov, Daniyar; Danilyan, Gevorg; Hutanu, Vladimir; Klenke, Jens; Masalovich, Sergey

2018-03-01

The TRI and ROT asymmetries in fission of heavy nuclei have been extensively studied during more than a decade. The effects were first discovered in the ternary fission in a series of experiments performed at the ILL reactor (Grenoble) by a collaboration of Russian and European institutes, and were carefully measured for a number of fissioning nuclei. Later on, the ROT effect has been observed in the emission of prompt gamma rays and neutrons in fission of 235U and 233U, although its value was an order of magnitude smaller than in the α-particle emission from ternary fission. All experiments performed so far are done with cold polarized neutrons, what assumes a mixture of several spin states, the weights of these states being not well known. The present paper describes the first attempt to get "clean" data by performing the measurement of gamma and neutron asymmetries in an isolated resonance of 235U at the POLI instrument of the FRM2 reactor in Garching.

Structure Of Neutron-Rich Nuclei In A˜100 Region Observed In Fusion-Fission Reactions

NASA Astrophysics Data System (ADS)

Wu, C. Y.; Hua, H.; Cline, D.; Hayes, A. B.; Teng, R.; Clark, R. M.; Fallon, P.; Görgen, A.; Macchiavelli, A. O.; Vetter, K.

2003-03-01

Neutron-rich nuclei around A˜100 were populated as fission fragments produced by the 238U(α,f) fusion-fission reaction. The deexcitation γ rays were detected by Gammasphere in coincidence with the detection of both fission fragments by the Rochester 4π heavy-ion detector array, CHICO. This technique allows Doppler-shift corrections to be applied for the observed γ rays on an event-by-event basis thus establishing the origin of γ rays from either fission fragment. In addition, it allows observation of γ-ray transitions from states with short lifetimes and offers the opportunity to study nuclear species beyond the reach of the spontaneous fission process. With these advantages, one can extend the spectroscopic study to higher spins than those derived using the thick-target technique, and to more neutron-rich nuclei than those derived from spontaneous fissions. Among the new and interesting phenomena identified in this rapid shape-changing region, the most distinct result is the evidence for a prolate-to-oblate shape transition occurring at 116Pd, which may have important implications to our understanding of the shell structure for neutron-rich nuclei.

Rotational Spin-up Caused CO2 Outgassing on Comet 103P/Hartley 2

NASA Astrophysics Data System (ADS)

Steckloff, Jordan; Graves, Kevin; Hirabayashi, Masatoshi; Richardson, James

2015-11-01

The Deep Impact spacecraft’s flyby of comet 103P/Hartley 2 on November 4, 2010 revealed its nucleus to be a small, bilobate, and highly active world [1] [2]. The bulk of this activity is driven by CO2 sublimation, which is enigmatically restricted to the tip of the small lobe [1]. Because Hartley 2's CO2 production responds to the diurnal cycle of the nucleus [1], CO2 ice must be no deeper than a few centimeters below the surface of the small lobe. However the high volatility of CO2 would suggest that its sublimation front should recede deep below the surface, such that diurnal volatile production is dominated by more refractory species such as water ice, as was observed at comet Tempel 1 [3].Here we show that both the near surface CO2 ice and its geographic restriction to the tip of the small lobe suggest that Hartley 2 recently experienced an episode of fast rotation. We use the GRAVMAP code to compute the stability of slopes on the surface of Hartley 2 as a function of spin period. We determine that the surface of the active region of Hartley 2’s small lobe becomes unstable at a rotation period of ~10-12 hours (as opposed to its current spin period of ~ 18 hours [1]), and will flow toward the tip of the lobe, excavating buried CO2 ice and activating CO2-driven activity. However, the rest of the surface of the nucleus is stable at these spin rates, and will therefore not exhibit CO2 activity. We additionally use Finite Element Model (FEM) analysis to demonstrate that the interior of Hartley 2’s nucleus is structurally stable (assuming a cohesive strength of at least 5 Pa) at these spin rates.The uncommonly high angular acceleration of Hartley 2, which has changed the nucleus spin period by two hours in three months [4], suggests that this episode of fast rotation may have existed only a few years or decades ago. Thus, Hartley 2 may provide an excellent case study into the reactivation of quiescent comet nuclei via rotational spin up, as would result from weak homogeneous gas emissions via the SYORP Effect.References: [1] A'Hearn et al. Science 332, 1396 (2011) [2] Thomas et al. Icarus 222, 550 (2013) [3] Feaga et al. Icarus 190, 345 (2007) [4] Samarasinha & Mueller. Ap. J. 775:L10 (2013)

Fission time scale from pre-scission neutron and α multiplicities in the 16O + 194Pt reaction

NASA Astrophysics Data System (ADS)

Kapoor, K.; Verma, S.; Sharma, P.; Mahajan, R.; Kaur, N.; Kaur, G.; Behera, B. R.; Singh, K. P.; Kumar, A.; Singh, H.; Dubey, R.; Saneesh, N.; Jhingan, A.; Sugathan, P.; Mohanto, G.; Nayak, B. K.; Saxena, A.; Sharma, H. P.; Chamoli, S. K.; Mukul, I.; Singh, V.

2017-11-01

Pre- and post-scission α -particle multiplicities have been measured for the reaction 16O+P194t at 98.4 MeV forming R210n compound nucleus. α particles were measured at various angles in coincidence with the fission fragments. Moving source technique was used to extract the pre- and post-scission contributions to the particle multiplicity. Study of the fission mechanism using the different probes are helpful in understanding the detailed reaction dynamics. The neutron multiplicities for this reaction have been reported earlier. The multiplicities of neutrons and α particles were reproduced using standard statistical model code joanne2 by varying the transient (τt r) and saddle to scission (τs s c) times. This code includes deformation dependent-particle transmission coefficients, binding energies and level densities. Fission time scales of the order of 50-65 ×10-21 s are required to reproduce the neutron and α -particle multiplicities.

Capture and fission with DANCE and NEUANCE

DOE PAGES

Jandel, M.; Baramsai, B.; Bond, E.; ...

2015-12-23

A summary of the current and future experimental program at DANCE is presented. Measurements of neutron capture cross sections are planned for many actinide isotopes with the goal to reduce the present uncertainties in nuclear data libraries. Detailed studies of capture gamma rays in the neutron resonance region will be performed in order to derive correlated data on the de-excitation of the compound nucleus. New approaches on how to remove the DANCE detector response from experimental data and retain the correlations between the cascade gamma rays are presented. Studies on 235U are focused on quantifying the population of short-lived isomericmore » states in 236U after neutron capture. For this purpose, a new neutron detector array NEUANCE is under construction. It will be installed in the central cavity of the DANCE array and enable the highly efficient tagging of fission and capture events. In addition, developments of fission fragment detectors are also underway to expand DANCE capabilities to measurements of fully correlated data on fission observables.« less

Capture and fission with DANCE and NEUANCE

NASA Astrophysics Data System (ADS)

Jandel, M.; Baramsai, B.; Bond, E.; Rusev, G.; Walker, C.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M. M.; Hayes, A.; Kawano, T.; Mosby, S.; Stetcu, I.; Taddeucci, T. N.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.

2015-12-01

A summary of the current and future experimental program at DANCE is presented. Measurements of neutron capture cross sections are planned for many actinide isotopes with the goal to reduce the present uncertainties in nuclear data libraries. Detailed studies of capture gamma rays in the neutron resonance region will be performed in order to derive correlated data on the de-excitation of the compound nucleus. New approaches on how to remove the DANCE detector response from experimental data and retain the correlations between the cascade gamma rays are presented. Studies on 235U are focused on quantifying the population of short-lived isomeric states in 236U after neutron capture. For this purpose, a new neutron detector array NEUANCE is under construction. It will be installed in the central cavity of the DANCE array and enable the highly efficient tagging of fission and capture events. In addition, developments of fission fragment detectors are also underway to expand DANCE capabilities to measurements of fully correlated data on fission observables.

The ^132Sn + ^96Zr reaction: a study of fusion enhancement/hindrance

NASA Astrophysics Data System (ADS)

Loveland, Walter; Vinodkumar, A. M.; Neeway, James; Sprunger, Peter; Prisbrey, Landon; Peterson, Donald; Liang, J. F.; Shapira, Dan; Gross, C. J.; Varner, R. L.; Kolata, J. J.; Roberts, A.; Caraley, A. L.

2008-10-01

Capture-fission cross sections were measured for the collision of the massive nucleus ^132Sn with ^96Zr at center of mass energies ranging from 192.8 to 249.6 MeV in an attempt to study fusion enhancement and hindrance in this reaction involving very neutron-rich nuclei. Coincident fission fragments were detected using silicon detectors. Using angle and energy conditions, deep inelastic scattering events were separated from fission events. Coupled channels calculations can describe the data if the surface diffuseness parameter, a, is allowed to be 1.10 fm, instead of the customary 0.6 fm. The measured capture-fission cross sections agree moderately well with model calculations using the dinuclear system (DNS) model. If we use this model to predict fusion barrier heights for these reactions, we find the predicted fusion hindrance, as represented by the extra push energy, is greater for the more neutron-rich system, lessening the advantage of the lower interaction barriers with neutron rich projectiles.

132Sn+96Zr reaction: A study of fusion enhancement/hindrance

NASA Astrophysics Data System (ADS)

Vinodkumar, A. M.; Loveland, W.; Neeway, J. J.; Prisbrey, L.; Sprunger, P. H.; Peterson, D.; Liang, J. F.; Shapira, D.; Gross, C. J.; Varner, R. L.; Kolata, J. J.; Roberts, A.; Caraley, A. L.

2008-11-01

Capture-fission cross sections were measured for the collision of the massive nucleus Sn132 with Zr96 at center-of-mass energies ranging from 192.8 to 249.6 MeV in an attempt to study fusion enhancement and hindrance in this reaction involving very neutron-rich nuclei. Coincident fission fragments were detected using silicon detectors. Using angle and energy conditions, deep inelastic scattering events were separated from fission events. Coupled-channels calculations can describe the data if the surface diffuseness parameter, a, is allowed to be 1.10 fm instead of the customary 0.6 fm. The measured capture-fission cross sections agree moderately well with model calculations using the dinuclear system model. If we use this model to predict fusion barrier heights for these reactions, we find the predicted fusion hindrance, as represented by the extra push energy, is greater for the more neutron-rich system, lessening the advantage of the lower interaction barriers with neutron-rich projectiles.

Asteroid Systems: Binaries, Triples, and Pairs

NASA Astrophysics Data System (ADS)

Margot, J.-L.; Pravec, P.; Taylor, P.; Carry, B.; Jacobson, S.

In the past decade, the number of known binary near-Earth asteroids has more than quadrupled and the number of known large main-belt asteroids with satellites has doubled. Half a dozen triple asteroids have been discovered, and the previously unrecognized populations of asteroid pairs and small main-belt binaries have been identified. The current observational evidence confirms that small (≲20 km) binaries form by rotational fission and establishes that the Yarkovsky-O'Keefe-Radzievskii-Paddack (YORP) effect powers the spin-up process. A unifying paradigm based on rotational fission and post-fission dynamics can explain the formation of small binaries, triples, and pairs. Large (>~20 km) binaries with small satellites are most likely created during large collisions.

Rapid evolution of the spin state of comet 41P/Tuttle-Giacobini-Kresak

NASA Astrophysics Data System (ADS)

Bodewits, Dennis; Farnham, Tony; Kelley, Michael S. P.; Manning Knight, Matthew

2018-01-01

Cometary outgassing can produce torques that change the spin state of the nucleus, influencing the evolution and lifetimes of comets. If these torques spin up the rotation to the point that centripetal forces exceed the material strength of the nucleus, the comet may fragment. Comet 41P/Tuttle-Giacobini-Kresak passed Earth as close as 0.142 au in April 2017, allowing observations of the inner coma and an assessment of the rotational state of the nucleus. We acquired observations of comet 41P between March and May 2017 using the 4.3-m Discovery Channel Telescope and the UltraViolet-Optical Telescope (UVOT) on board the Earth-orbiting Swift Gamma Ray Burst Mission.We combined CN narrowband imaging and aperture photometry and found that the apparent rotation period of comet 41P more than doubled between March and May 2017, increasing from 20 hours to over 46 hours. Measurements of the periodicity in late-March by Knight et al. (CBET 4377, 2017) are consistent with this rate of increase. Comet 41P is the ninth comet for which a rotation period change has been observed (c.f. Samarasinha et al., in Comets II, 2004), but both the fractional change and the rate of change of the period far exceed those observed in the other comets. It is the combination of a slow rotation, high activity, and a small nucleus that contribute to the rapid changes of the rotation state of 41P. In addition, the active regions on the surface of 41P are likely oriented in a way such that its torques are highly optimized in comparison to many other comets.Extrapolating the comet’s rotation period using its current gas production rates and a simple activity model suggests that the nucleus will continue to spin down, possibly leading to an excited spin state in the next apparitions. Finally, 41P is known for its large outbursts, and our extrapolation suggest that the comet’s rotation period may have been close to the critical period for splitting in 2001, when it exhibited two significant outbursts.

Long-Lived Correlated Triplet Pairs in a π-Stacked Crystalline Pentacene Derivative.

PubMed

Folie, Brendan D; Haber, Jonah B; Refaely-Abramson, Sivan; Neaton, Jeffrey B; Ginsberg, Naomi S

2018-02-14

Singlet fission is the spin-conserving process by which a singlet exciton splits into two triplet excitons. Singlet fission occurs via a correlated triplet pair intermediate, but direct evidence of this state has been scant, and in films of TIPS-pentacene, a small molecule organic semiconductor, even the rate of fission has been unclear. We use polarization-resolved transient absorption microscopy on individual crystalline domains of TIPS-pentacene to establish the fission rate and demonstrate that the initially created triplets remain bound for a surprisingly long time, hundreds of picoseconds, before separating. Furthermore, using a broadband probe, we show that it is possible to determine absorbance spectra of individual excited species in a crystalline solid. We find that triplet interactions perturb the absorbance, and provide evidence that triplet interaction and binding could be caused by the π-stacked geometry. Elucidating the relationship between the lattice structure and the electronic structure and dynamics has important implications for the creation of photovoltaic devices that aim to boost efficiency via singlet fission.

Experimental evidence for 56Ni-core breaking from the low-spin structure of the N=Z nucleus 5829Cu29

NASA Astrophysics Data System (ADS)

Lisetskiy, A. F.; Pietralla, N.; Honma, M.; Schmidt, A.; Schneider, I.; Gade, A.; von Brentano, P.; Otsuka, T.; Mizusaki, T.; Brown, B. A.

2003-09-01

Low-spin states in the odd-odd N=Z nucleus 58Cu were investigated with the 58Ni(p,nγ)58Cu fusion evaporation reaction at the FN-TANDEM accelerator in Cologne. γγ-coincidences, γγ-angular correlations, and signs of γ-ray polarizations were measured. Seventeen low-spin states below 3.6 MeV and 17 new transitions were observed. Ten multipole mixing ratios and 17 γ-branching ratios were determined for the first time. New detailed spectroscopic information on the 2+2 state, the isobaric analogue state (IAS) of the 2+1,T=1 state of 58Ni, makes 58Cu the heaviest odd-odd N=Z nucleus with known B(E2;2+,T=1→0+,T=1) value. The 4+ state at 2.751 MeV, observed here for the first time, is identified as the IAS of the 4+1,T=1 state in 58Ni. The new data are compared to full pf-shell-model calculations with the GXPF1 residual interaction and to calculations within a pf5/2 configurational space with a residual surface δ interaction. The role of the 56Ni core excitations for the low-spin structure in 58Cu is discussed.

Singlet-Fission-Sensitized Hybrid Thin-Films For Next-Generation Photovoltaics

DTIC Science & Technology

2016-04-12

evaporators and a spin-coater was constructed. In order to characterize PV devices, a solar -simulator, 1. REPORT DATE (DD-MM-YYYY) 4. TITLE AND...with thermal evaporators and a spin-coater was constructed. In order to characterize PV devices, a solar -simulator, semiconductor parameter analyzer...SECURITY CLASSIFICATION OF: This grant enabled the acquisition of equipment for the fabrication of organic and nanocrystal based photovoltaic ( PV

Isotope-Identifying neutron reflectometry

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nikitenko, Yu. V., E-mail: nikiten@nf.jinr.ru; Petrenko, A. V.; Gundorin, N. A.

2015-07-15

The possibilities of an isotope-indentifying study of layered structures in different regimes of a neutron wave field are considered. The detection of specularly reflected neutrons and secondary radiation (caused by neutron capture) in the form of charged particles, γ quanta, and nuclear fission fragments, as well as neutrons spin-flipped in a noncollinear magnetic field and on nuclei of elements with spin, makes it possible to implement isotope-indentifying neutron reflectometry.

Sensitivity of the nuclear deformability and fission barriers to the equation of state

NASA Astrophysics Data System (ADS)

Seif, W. M.; Anwer, Hisham

2018-07-01

The model-dependent analysis of the fission data impacts the extracted fission-related quantities, which are not directly observables, such as the super- and hyperdeformed isomeric states and their energies. We investigated the model dependence of the deformability of a nucleus and its fission barriers on the nuclear equation of state. Within the microscopic-macroscopic model based on a large number of Skyrme nucleon-nucleon interactions, the total energy surfaces and the double-humped fission barrier of 230Th are calculated in a multidimensional deformation space. In addition to the ground-state (GS) and the superdeformed (SD) minima, all the investigated forces yielded a hyperdeformed (HD) minimum. The contour map of the shell-plus-pairing energy clearly displayed the three minima. We found that the GS binding energy and the deformation energy of the different deformation modes along the fission path increase with the incompressibility coefficient K0, while the fission barrier heights and the excitation energies of the SD and HD modes decrease with it. Conversely, the surface-energy coefficient asurf, the symmetry-energy, and its density-slope parameter decrease the GS energy and the deformation energies, but increase the fission barrier heights and the excitation energies. The obtained deformation parameters of the different deformation modes exhibit almost independence on K0, and on the symmetry-energy and its density-slope. The principle deformation parameters of the SD and HD isomeric states tend to decrease with asurf.

Table of superdeformed nuclear bands and fission isomers (from Nuclear Data Sheets, v.78, issue 1, May 1996)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Singh, B.; Firestone, R B.; Chu, S Y.F.

As part of a committment to maintain nuclear structure data as current as possible in the Evaluated Nuclear Structure Data File (ENSDF) and the Table of Isotopes, the author have been updating the information on superdeformed and hyperdeformed nuclear bands. As of February, 1996, they have compiled data for 161 superdeformed bands and 47 fission isomers identified in 93 nuclides for this publication. This is an increase of 75 superdeformed bands and 20 new nuclides since the first edition in 1994. Partial data for superdeformed bands and fission isomers are shown in the band drawings. For each nuclide there ismore » a complete level table listing both normal (taken from the ENSDF file) and superdeformed band assignments; level energy, spin, parity, half-life, magnetic moments, decay branchings; and the energies, final levels, relative intensities, multipolarities, and mixing ratios for transitions deexciting each level. Mass excess, decay energies, and proton and neutron separation energies are also provided from the evaluation of Audi and Wapstra. For superdeformed and hyperdeformed bands they provide the following quantities: level energies; level half-lives; level spins; and gamma ray energies.« less

A Study of Primary Collision Dynamics in Inverse-Kinematics Reaction of 78Kr on 40Ca at a Bombarding Energy of 10 MeV per Nucleon

NASA Astrophysics Data System (ADS)

Henry, Eric M.

The CHIMERA multi-detector array at LNS Catania has been used to study the inverse-kinematics reaction of 78Kr + 40Ca at a bombarding energy of 10 A MeV. The multi-detector is capable of detecting individual products of the collision essential for the reconstruction of the collision dynamics. This is the first time CHIMERA has been used at low-energy, which offered a unique challenge for the calibration and interpretation of experimental data. Initial interrogation of the calibrated data revealed a class of selected events characterized by two coincident heavy fragments (atomic number Z>3) that together account for the majority of the total mass of the colliding system. These events are consistent with the complete fusion and subsequent binary split (fission) of a composite nucleus. The observed fission fragments are characterized by a broad A, Z distribution and are centered about symmetric fission while exhibiting relative velocities significantly higher than given by Viola systematics. Additional analysis of the kinematic relationship between the fission fragments was performed. Of note, is that the center-of-mass angular distribution (dsigma/dtheta) of the fission fragments exhibits an unexpected anisotropy inconsistent with a compound-nucleus reaction. This anisotropy is indicative of a dynamic fusion/fission-like process. The observed angular distribution features a forward-backward anisotropy most prevalent for mass-asymmetric events. Furthermore, the more massive fragment of mass-asymmetric events appears to emerge preferentially in the forward direction, along the beam axis. Analysis of the angular distribution of alpha particles emitted from these fission fragments suggests the events are associated mostly with central collisions. The observations associated with this subset of events are similar to those reported for dynamic fragmentation of projectile-like fragments, but have not before been observed for a fusion/fission-like process. Comparisons to dynamic and statistical reaction model predictions are inconsistent with known phenomena, but suggest a peculiar dynamics-driven scenario. A plausible explanation of the experimental results is the existence of a phenomenon similar to a "fusion window", or a range of impact parameters in which complete fusion cannot be achieved. In this scenario, the system must absorb all the relative motion and convert it to vibrational energy or heat. As the energy increases the system may not be able to accommodate this conversion of energy without breaking apart.

Phospholipid bilayer relaxation dynamics as revealed by the pulsed electron-electron double resonance of spin labels

NASA Astrophysics Data System (ADS)

Syryamina, V. N.; Dzuba, S. A.

2012-10-01

Electron paramagnetic resonance (EPR) spectroscopy in the form of pulsed electron-electron double resonance (ELDOR) was applied to 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphocholine (POPC) phospholipid bilayers containing lipids that were spin-labeled at different carbon positions along the lipid acyl chain. Pulsed ELDOR detects motionally induced spin flips of nitrogen nuclei in the nitroxide spin labels, which manifests itself as magnetization transfer (MT) in the nitroxide EPR spectrum. The MT effect was observed over a wide temperature range (100-225 K) on a microsecond time scale. In line with a previous study on molecular glasses [N. P. Isaev and S. A. Dzuba, J. Chem. Phys. 135, 094508 (2011), 10.1063/1.3633241], the motions that induce MT effect were suggested to have the same nature as those in dielectric secondary (β) Johari-Goldstein fast relaxation. The results were compared with literature dielectric relaxation data for POPC bilayers, revealing some common features. Molecular motions resulting in MT are faster for deeper spin labels in the membrane interior. The addition of cholesterol to the bilayer suppresses the lipid motions near the steroid nucleus and accelerates the lipid motions beyond the steroid nucleus, in the bilayer interior. This finding was attributed to the lipid acyl chains being more ordered near the steroid nucleus and less ordered in the bilayer interior. The motions are absent in dry lipids, indicating that the motions are determined by intermolecular interactions in the bilayer.

Nuclear Propulsion for Space Applications

NASA Technical Reports Server (NTRS)

Houts, M. G.; Bechtel, R. D.; Borowski, S. K.; George, J. A.; Kim, T.; Emrich, W. J.; Hickman, R. R.; Broadway, J. W.; Gerrish, H. P.; Adams, R. B.

2013-01-01

Basics of Nuclear Systems: Long history of use on Apollo and space science missions. 44 RTGs and hundreds of RHUs launched by U.S. during past 4 decades. Heat produced from natural alpha (a) particle decay of Plutonium (Pu-238). Used for both thermal management and electricity production. Used terrestrially for over 65 years. Fissioning 1 kg of uranium yields as much energy as burning 2,700,000 kg of coal. One US space reactor (SNAP-10A) flown (1965). Former U.S.S.R. flew 33 space reactors. Heat produced from neutron-induced splitting of a nucleus (e.g. U-235). At steady-state, 1 of the 2 to 3 neutrons released in the reaction causes a subsequent fission in a "chain reaction" process. Heat converted to electricity, or used directly to heat a propellant. Fission is highly versatile with many applications.

Bruyères-le-Châtel Neutron Evaluations of Actinides with the TALYS Code: The Fission Channel

DOE Office of Scientific and Technical Information (OSTI.GOV)

Romain, P., E-mail: pascal.romain@cea.fr; Morillon, B.; Duarte, H.

For several years, various neutron evaluations of plutonium and uranium isotopes have been performed at Bruyères-le-Châtel (BRC), from 1 keV up to 30 MeV. Since only nuclear reaction models have been used to produce these evaluations, our approach was named the “Full Model” approach. Total, shape elastic and direct inelastic cross sections were obtained from the coupled channels model using a dispersive optical potential developed for actinides, with a large enough coupling scheme including the lowest octupolar band. All other cross sections were calculated using the Hauser-Feshbach theory (TALYS code) with a pre-equilibrium component above 8–10 MeV. In this paper,more » we focus our attention on the fission channel. More precisely, we will present the BRC contribution to fission modeling and the philosophy adopted in our “Full Model” approach. Performing evaluations with the “Full Model” approach implies the optimization of a large number of model parameters. With increasing neutron incident energy, many residual nuclei produced by nucleon emission also lead to fission. All available experimental data assigned to various fission mechanisms of the same nucleus were used to determine fission barrier parameters. For uranium isotopes, triple-humped fission barriers were required in order to reproduce accurately variations of the experimental fission cross sections. Our BRC fission modeling has shown that the effects of the class II or class III states located in the wells of the fission barrier sometimes provide an anti-resonant transmission rather than a resonant one. Consistent evaluations were produced for a large series of U and Pu isotopes. Resulting files were tested against integral data.« less

A Cytoplasmic Dynein Heavy Chain Is Required for Oscillatory Nuclear Movement of Meiotic Prophase and Efficient Meiotic Recombination in Fission Yeast

PubMed Central

Yamamoto, Ayumu; West, Robert R.; McIntosh, J. Richard; Hiraoka, Yasushi

1999-01-01

Meiotic recombination requires pairing of homologous chromosomes, the mechanisms of which remain largely unknown. When pairing occurs during meiotic prophase in fission yeast, the nucleus oscillates between the cell poles driven by astral microtubules. During these oscillations, the telomeres are clustered at the spindle pole body (SPB), located at the leading edge of the moving nucleus and the rest of each chromosome dangles behind. Here, we show that the oscillatory nuclear movement of meiotic prophase is dependent on cytoplasmic dynein. We have cloned the gene encoding a cytoplasmic dynein heavy chain of fission yeast. Most of the cells disrupted for the gene show no gross defect during mitosis and complete meiosis to form four viable spores, but they lack the nuclear movements of meiotic prophase. Thus, the dynein heavy chain is required for these oscillatory movements. Consistent with its essential role in such nuclear movement, dynein heavy chain tagged with green fluorescent protein (GFP) is localized at astral microtubules and the SPB during the movements. In dynein-disrupted cells, meiotic recombination is significantly reduced, indicating that the dynein function is also required for efficient meiotic recombination. In accordance with the reduced recombination, which leads to reduced crossing over, chromosome missegregation is increased in the mutant. Moreover, both the formation of a single cluster of centromeres and the colocalization of homologous regions on a pair of homologous chromosomes are significantly inhibited in the mutant. These results strongly suggest that the dynein-driven nuclear movements of meiotic prophase are necessary for efficient pairing of homologous chromosomes in fission yeast, which in turn promotes efficient meiotic recombination. PMID:10366596

Magnitude of finite-nucleus-size effects in relativistic density functional computations of indirect NMR nuclear spin-spin coupling constants.

PubMed

Autschbach, Jochen

2009-09-14

A spherical Gaussian nuclear charge distribution model has been implemented for spin-free (scalar) and two-component (spin-orbit) relativistic density functional calculations of indirect NMR nuclear spin-spin coupling (J-coupling) constants. The finite nuclear volume effects on the hyperfine integrals are quite pronounced and as a consequence they noticeably alter coupling constants involving heavy NMR nuclei such as W, Pt, Hg, Tl, and Pb. Typically, the isotropic J-couplings are reduced in magnitude by about 10 to 15 % for couplings between one of the heaviest NMR nuclei and a light atomic ligand, and even more so for couplings between two heavy atoms. For a subset of the systems studied, viz. the Hg atom, Hg(2) (2+), and Tl--X where X=Br, I, the basis set convergence of the hyperfine integrals and the coupling constants was monitored. For the Hg atom, numerical and basis set calculations of the electron density and the 1s and 6s orbital hyperfine integrals are directly compared. The coupling anisotropies of TlBr and TlI increase by about 2 % due to finite-nucleus effects.

Electron Spin Resonance (ESR) Studies of Returned Comet Nucleus Samples

NASA Technical Reports Server (NTRS)

Tsay, Fun-Dow; Kim, Soon Sam; Liang, Ranty H.

1997-01-01

Electron Spin Resonance (ESR) studies have been carried out on organic and inorganic free radicals generated by gamma-ray and/or UV-irradiation and trapped in ice matrices. It is suggested that the concentration of these free radicals together with their thermal stability can be used as an accurate built-in geothermometer and radiation probe for returned comet nucleus sample studies. ESR studies have also been carried out on paramagnetic (Mn(2+), Ti(3+), and Fe(3+)) and ferromagnetic (ferric oxide and metallic iron) centers known to be present in terrestrial and extraterrestrial samples. The presence or absence of these magnetic centers coupled with their characteristic ESR lineshape can be used to investigate the shock effects, quenching/cooling rate and oxidation-reduction conditions in the formation and subsequent evolution of returned comet nucleus samples.

Measurement of Plutonium-240 Angular Momentum Dependent Fission Probabilities Using the Alpha-Alpha' Reaction

NASA Astrophysics Data System (ADS)

Koglin, Johnathon

Accurate nuclear reaction data from a few keV to tens of MeV and across the table of nuclides is essential to a number of applications of nuclear physics, including national security, nuclear forensics, nuclear astrophysics, and nuclear energy. Precise determination of (n, f) and neutron capture cross sections for reactions in high- ux environments are particularly important for a proper understanding of nuclear reactor performance and stellar nucleosynthesis. In these extreme environments reactions on short-lived and otherwise difficult-to-produce isotopes play a significant role in system evolution and provide insights into the types of nuclear processes taking place; a detailed understanding of these processes is necessary to properly determine cross sections far from stability. Indirect methods are often attempted to measure cross sections on isotopes that are difficult to separate in a laboratory setting. Using the surrogate approach, the same compound nucleus from the reaction of interest is created through a "surrogate" reaction on a different isotope and the resulting decay is measured. This result is combined with appropriate reaction theory for compound nucleus population, from which the desired cross sections can be inferred. This method has shown promise, but the theoretical framework often lacks necessary experimental data to constrain models. In this work, dual arrays of silicon telescope particle identification detectors and photovoltaic (solar) cell fission fragment detectors have been used to measure the fission probability of the 240Pu(alpha, alpha'f) reaction - a surrogate for the 239Pu(n, f) - and fission of 35.9(2)MeV at eleven scattering angles from 40° to 140° in 10° intervals and at nuclear excitation energies up to 16MeV. Within experimental uncertainty, the maximum fission probability was observed at the neutron separation energy for each alpha scattering angle. Fission probabilities were separated into five 500 keV bins from 5:5MeV to 8:0MeV and one bin from 4:5MeV to 5:5MeV. Across energy bins the fission probability increases approximately linearly with increasing alpha' scattering angle. At 90° the fission probability increases from 0:069(6) in the lowest energy bin to 0:59(2) in the highest. Likewise, within a single energy bin the fission probability increases with alpha' scattering angle. Within the 6:5MeV and 7:0MeV energy bin, the fission probability increased from 0:41(1) at 60° to 0:81(10) at 140°. Fission fragment angular distributions were also measured integrated over each energy bin. These distributions were fit to theoretical distributions based on combinations of transitional nuclear vibrational and rotational excitations at the saddle point. Contributions from specific K vibrational states were extracted and combined with fission probability measurements to determine the relative fission probability of each state as a function of nuclear excitation energy. Within a given excitation energy bin, it is found that contributions from K states greater than the minimum K = 0 state tend to increase with the increasing alpha' scattering angle. This is attributed to an increase in the transferred angular momentum associated with larger scattering angles. The 90° alpha' scattering angle produced the highest quality results. The relative contributions of K states do not show a discernible trend across the energy spectrum. The energy-binned results confirm existing measurements that place a K = 2 state in the first energy bin with the opening of K = 1 and K = 4 states at energies above 5:5MeV. This experiment represents the first of its kind in which fission probabilities and angular distributions are simultaneously measured at a large number of scattering angles. The acquired fission probability, angular distribution, and K state contribution provide a diverse dataset against which microscopic fission models can be constrained and further the understanding of the properties of the 240Pu fission.

A new analysis of archival images of comet 29P/Schwassmann-Wachmann 1 to constrain the rotation state of and active regions on its nucleus

NASA Astrophysics Data System (ADS)

Schambeau, C.; Fernández, Y.; Samarasinha, N.; Mueller, B.; Woodney, L.; Lisse, C.; Kelley, M.; Meech, K.

2014-07-01

Introduction: 29P/Schwassmann-Wachmann 1 (SW1) is a unique comet (and Centaur) with an almost circular orbit just outside the orbit of Jupiter. This orbit results in SW1 receiving a nearly constant insolation, thus giving a simpler environment in which to study thermal properties and behaviors of this comet's nucleus. Such knowledge is crucial for improving our understanding of coma morphology, nuclear thermal evolution, and nuclear structure. To this end, our overarching goal is to develop a thermophysical model of SW1's nucleus that makes use of realistic physical and structural properties as inputs. This model will help to explain the highly variable gas- and dust-production rates of this comet; SW1 is well known for its frequent but stochastic outbursts of mass loss [1,2,3]. Here we will report new constraints on the effective radius, beaming parameter, spin state, and location of active regions on the nucleus of SW1. Results: The analysis completed so far consists of a re-analysis of Spitzer Space Telescope thermal-IR images of SW1 from UT 2003 November 21 and 24, when SW1 was observed outside of outburst. The images are from Spitzer's IRAC 5.8-μm and 8.0-μm bands and MIPS 24.0-μm and 70-μm bands. This analysis is similar to that of Stansberry et al. [4, 5], but with data products generated from the latest Spitzer pipeline. Also, analysis of the 5.8-μm image had not been reported before. Coma removal techniques (e.g., Fernández et al. [6]) were applied to each image letting us measure the nuclear point-source contribution to each image. The measured flux densities for each band were fit with a Near Earth Asteroid Thermal Model (NEATM, [7]) and resulted in values for the effective radius of SW1's nucleus, constraints on the thermal inertia, and an IR beaming-parameter value. Current efforts have shifted to constraining the spin properties of SW1's nucleus and surface areas of activity through use of an existing Monte Carlo model [8, 9] to reproduce existing images (in our possession) of SW1's dust coma while in and out of outburst. The images analyzed so far consist of R-band (CCD) images of SW1 taken with the Kitt Peak National Observatory 2.1-m telescope on Sept. 25.5, 26.5, 27.5, 28.5, and 29.5 UT in 2008 [10]. SW1 was undergoing an outburst during this time and showed three continuous radial jets of material as well as at least one and possibly two expanding shells, all of which may let us constrain the active areas and the spin properties of the nucleus. By using the nucleus's spin state, location and extent of active areas, and dust-grain velocities as inputs to the model, we will mimic the observed coma morphology. Using this technique, we will present constraints to the nuclear properties of SW1. It is expected that due to the large size of SW1's nucleus measured earlier, any rotational excitation of the nucleus would/should have damped to a principal-axis spin state, simplifying our modeling efforts. The coma modeling will also enable us to examine this assumption.

Experimental study of the β decay of the very neutron-rich nucleus Ge 85

DOE PAGES

Korgul, A.; Rykaczewski, Krzysztof Piotr; Grzywacz, Robert Kazimierz; ...

2017-04-04

The β -decay properties of the very neutron-rich nucleus 85Ge, produced in the proton-induced fission of 238U, were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. The level scheme of 33 85As 52 populated in 85Geβ γ decay was reconstructed and compared to shell-model calculations. The investigation of the systematics of low-energy levels in N =52 isotones together with shell-model analysis allowed us to provide an estimate of the low-energy structure of the more exotic N =52 isotone 81Cu.

FAST ROTATION AND TRAILING FRAGMENTS OF THE ACTIVE ASTEROID P/2012 F5 (GIBBS)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Drahus, Michał; Waniak, Wacław; Tendulkar, Shriharsh

While having a comet-like appearance, P/2012 F5 (Gibbs) has an orbit native to the Main Asteroid Belt, and physically is a km-sized asteroid which recently (mid 2011) experienced an impulsive mass ejection event. Here we report new observations of this object obtained with the Keck II telescope on UT 2014 August 26. The data show previously undetected 200 m scale fragments of the main nucleus, and reveal a rapid nucleus spin with a rotation period of 3.24 ± 0.01 hr. The existence of large fragments and the fast nucleus spin are both consistent with rotational instability and partial disruption ofmore » the object. To date, many fast rotators have been identified among the minor bodies, which, however, do not eject detectable fragments at the present-day epoch, and also fragmentation events have been observed, but with no rotation period measured. P/2012 F5 is unique in that for the first time we detected fragments and quantified the rotation rate of one and the same object. The rapid spin rate of P/2012 F5 is very close to the spin rates of two other active asteroids in the Main Belt, 133P/Elst-Pizarro and (62412), confirming the existence of a population of fast rotators among these objects. But while P/2012 F5 shows impulsive ejection of dust and fragments, the mass loss from 133P is prolonged and recurrent. We believe that these two types of activity observed in the rapidly rotating active asteroids have a common origin in the rotational instability of the nucleus.« less

Probing the effect of neutron excess on the dynamics of Hf compound system

NASA Astrophysics Data System (ADS)

Sharma, Ishita; Kumar, Raj; Sharma, Manoj K.

2018-05-01

The reaction dynamics of 170Hf* and 174Hf* compound systems formed in 46,50Ti +124Sn reactions have been analyzed within the framework of Dynamical Cluster-decay Model (DCM) over an energy range of Ec.m.=115-156 MeV. The experimental data of fusion evaporation cross sections for 170,174Hf* systems is successfully addressed by optimizing the value of neck length ΔR. It is to be noted that calculations are performed by taking quadrupole deformations β2 with the optimum orientation of decaying fragments. Here, the effect of neutron excess has been examined on the structural properties of decaying fragments via fragmentation potential and preformation probability. The observation depicts that the isotopic effect prevails at fission region and as we move from lighter nucleus i.e. 170Hf* to heavier nucleus i.e. 174Hf*, the heavy mass fragments (HMF) start contributing along with fission fragments which are equally evident for 170Hf* as well. The ΔR values so obtained are compared at center of mass-energies which consequently provides information regarding the relative time scale of decaying fragments.

The Rate of Decay of Fission Products

DOE PAGES

May, K.; Wigner, Eugene P.

1948-06-01

By considering the fission products as a sort of statistical assembly, calculations have been made of the β -disintegrations per second and of the total energy emitted per second at any time after fission has taken place (cf. Fig. 6). The results are in good agreement with experiment. The theoretical work is based on the assumption that the mass of a nucleus of mass number A and charge Z is given by a ( Z 0 ( A ) - Z ) 2 + b . Empirical values for a and b are used. Use is also made of anmore » approximate empirical relationship between half-life and disintegration energy. A further basic hypothesis which is important for the results at very short times after fission has taken place is that, in the most probable way of splitting, the chain lengths of the light and heavy fragments are equal and that there is not much deviation from this most probable mode of fission. (See L. E. Glendenin, C. D. Coryell, R. R. Edwards, and M. H. Feldman, CL-LEG-1. A tentative explanation has been given recently by R. D. Present, Phys. Rev. 72, 7 (1947).) The average number of β -disintegrations per fission is found to be 6; the average energy of all radiations ( β, γ, and neutrino) of the fission products is 21.5 ± 3 Mev. Apparently, about half of this energy escapes in the form of neutrinos and a quarter is emitted in the form of β and in the form of γ rays.« less

Fusion-fission Study at JAEA for Heavy-element Synthesis

NASA Astrophysics Data System (ADS)

Nishio, K.

Fission fragment mass distributions were measured in the heavy-ion induced fission using 238U target nucleus. The mass distribu- tions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and qasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their inci- dent energy dependence. Fusion probability was determined in the analysis. Evaporation residue cross sections were calculated with a statistical model in the reactions of 30Si+238U and 34S+238U using the obtained fusion probability in the entrance channel. The results agree with the measured cross sections of 263,264Sg and 267,268Hs, produced by 30Si+238U and 34S+238U, respectively. It is also suggested that the sub-barrier energies can be used for heavy element synthesis.

Decay and Fission Hindrance of Two- and Four-Quasiparticle K Isomers in Rf 254

DOE Office of Scientific and Technical Information (OSTI.GOV)

David, H. M.; Chen, J.; Seweryniak, D.

2015-09-01

Two isomers decaying by electromagnetic transitions with half-lives of 4.7(1.1) and 247 ( 73 ) μ s have been discovered in the heavy 254 Rf nucleus. The observation of the shorter-lived isomer was made possible by a novel application of a digital data acquisition system. The isomers were interpreted as the K π = 8 - , ν 2 ( 7 / 2 + [ 624 ] , 9 / 2 - [ 734 ] ) two-quasineutron and the K π = 1 6 + , 8 - ν 2 ( 7 / 2 + [ 624 ] , 9more » / 2 - [ 734 ] ) Ⓧ 8 - π 2 ( 7 / 2 -[ 514 ] , 9 / 2 + [ 624 ] ) four-quasiparticle configurations, respectively. Surprisingly, the lifetime of the two-quasiparticle isomer is more than 4 orders of magnitude shorter than what has been observed for analogous isomers in the lighter N = 150 isotones. The four-quasiparticle isomer is longer lived than the 254 Rf ground state that decays exclusively by spontaneous fission with a half-life of 23.2 ( 1.1 ) μ s . The absence of sizable fission branches from either of the isomers implies unprecedented fission hindrance relative to the ground state.« less

Decay and Fission Hindrance of Two- and Four-Quasiparticle K Isomers in ^{254}Rf.

PubMed

David, H M; Chen, J; Seweryniak, D; Kondev, F G; Gates, J M; Gregorich, K E; Ahmad, I; Albers, M; Alcorta, M; Back, B B; Baartman, B; Bertone, P F; Bernstein, L A; Campbell, C M; Carpenter, M P; Chiara, C J; Clark, R M; Cromaz, M; Doherty, D T; Dracoulis, G D; Esker, N E; Fallon, P; Gothe, O R; Greene, J P; Greenlees, P T; Hartley, D J; Hauschild, K; Hoffman, C R; Hota, S S; Janssens, R V F; Khoo, T L; Konki, J; Kwarsick, J T; Lauritsen, T; Macchiavelli, A O; Mudder, P R; Nair, C; Qiu, Y; Rissanen, J; Rogers, A M; Ruotsalainen, P; Savard, G; Stolze, S; Wiens, A; Zhu, S

2015-09-25

Two isomers decaying by electromagnetic transitions with half-lives of 4.7(1.1) and 247(73) μs have been discovered in the heavy ^{254}Rf nucleus. The observation of the shorter-lived isomer was made possible by a novel application of a digital data acquisition system. The isomers were interpreted as the K^{π}=8^{-}, ν^{2}(7/2^{+}[624],9/2^{-}[734]) two-quasineutron and the K^{π}=16^{+}, 8^{-}ν^{2}(7/2^{+}[624],9/2^{-}[734])⊗8^{-}π^{2}(7/2^{-}[514],9/2^{+}[624]) four-quasiparticle configurations, respectively. Surprisingly, the lifetime of the two-quasiparticle isomer is more than 4 orders of magnitude shorter than what has been observed for analogous isomers in the lighter N=150 isotones. The four-quasiparticle isomer is longer lived than the ^{254}Rf ground state that decays exclusively by spontaneous fission with a half-life of 23.2(1.1) μs. The absence of sizable fission branches from either of the isomers implies unprecedented fission hindrance relative to the ground state.

Lifetime measurements in shape transition nucleus 188Pt

NASA Astrophysics Data System (ADS)

Rohilla, Aman; Gupta, C. K.; Singh, R. P.; Muralithar, S.; Chakraborty, S.; Sharma, H. P.; Kumar, A.; Govil, I. M.; Biswas, D. C.; Chamoli, S. K.

2017-04-01

Nuclear level lifetimes of high spin states in yrast and non-yrast bands of 188Pt nucleus have been measured using recoil distance plunger setup present at IUAC, Delhi. In the experiment nuclear states of interest were populated via 174Yb(18O,4 n)188Pt reaction at a beam energy of 79MeV provided by 15 UD Pelletron accelerator. The extracted B(E2\\downarrow) values show an initial rise up to 4+ state and then a nearly constant behavior with spin along yrast band, indicating change of nuclear structure in 188Pt at low spins. The good agreement between experimental and TPSM model B(E2\\downarrow) values up to 4^+ state suggests an increase in axial deformation of the nucleus. The average absolute β2 = 0.20 (3) obtained from measured B(E2\\downarrow) values matches well the values predicted by CHFB and IBM calculations for oblate ( β2 ˜ -0.19) and prolate (β2 ˜ 0.22) shapes. As the lifetime measurements do not yield the sign of β2, no definite conclusion can be drawn on the prolate or oblate collectivity of 188Pt on the basis of present measurements.

Positive parity low spin states of odd-mass tellurium isotopes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yazar, Harun Resit

2006-11-15

In this work, we analyse the positive parity of states of odd-mass nucleus within the framework of interacting boson fermion model. The result of an IBFM-1 multilevel calculation with the lg{sub 9/2}, 2d{sub 5/2}, 2d{sub 3/2}, 3s{sub 1/2} and one level, 1h{sub 11/2} with negative parity, single particle orbits is reported for the positive parity states of the odd mass nucleus {sup 123-125}Te. Also, an IBM-1 calculation is presented for the low-lying states in the even-even {sup 124-126}Te core nucleus. The energy levels and B (E2) transition probabilities were calculated and compared with the experimental data. It was found thatmore » the calculated positive parity low spin state energy spectra of the odd-mass {sup 123-125}Te isotopes agree quite well with the experimental data.« less

Revised and extended level scheme of the doubly-odd nucleus {sup 188}Ir

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jungclaus, A.; Modamio, V.; Egido, J. L.

2008-02-15

High-spin states in the doubly odd Z=77 nucleus {sup 188}Ir were studied using the reaction {sup 186}W({sup 7}Li, 5n) at 59 MeV and the GASP spectrometer for {gamma}-ray detection. The level structures recently suggested to be built on the known 4.1(3) ms isomeric state of this nucleus have been considerably revised and extended and an isomer with a lifetime of 17.7(2) ns has been identified within the main decay sequence. In addition two rotational bands built on low spin states below the ms isomer have been observed for the first time. The basic features of the excitation scheme of {supmore » 188}Ir are discussed within the Hartree-Fock-Bogoliubov theory within the Lipkin-Nogami approach with the finite-range density-dependent Gogny force.« less

External quantum efficiency exceeding 100% in a singlet-exciton-fission-based solar cell

NASA Astrophysics Data System (ADS)

Baldo, Marc

2013-03-01

Singlet exciton fission can be used to split a molecular excited state in two. In solar cells, it promises to double the photocurrent from high energy photons, thereby breaking the single junction efficiency limit. We demonstrate organic solar cells that exploit singlet exciton fission in pentacene to generate more than one electron per incident photon in the visible spectrum. Using a fullerene acceptor, a poly(3-hexylthiophene) exciton confinement layer, and a conventional optical trapping scheme, the peak external quantum efficiency is (109 +/-1)% at λ = 670 nm for a 15-nm-thick pentacene film. The corresponding internal quantum efficiency is (160 +/-10)%. Independent confirmation of the high internal efficiency is obtained by analysis of the magnetic field effect on photocurrent, which determines that the triplet yield approaches 200% for pentacene films thicker than 5 nm. To our knowledge, this is the first solar cell to generate quantum efficiencies above 100% in the visible spectrum. Alternative multiple exciton generation approaches have been demonstrated previously in the ultraviolet, where there is relatively little sunlight. Singlet exciton fission differs from these other mechanisms because spin conservation disallows the usual dominant loss process: a thermal relaxation of the high-energy exciton into a single low-energy exciton. Consequently, pentacene is efficient in the visible spectrum at λ = 670 nm because only the collapse of the singlet exciton into twotriplets is spin-allowed. Supported as part of the Center for Excitonics, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001088.

High-spin lifetime measurements in the N=Z nucleus Kr72

NASA Astrophysics Data System (ADS)

Andreoiu, C.; Svensson, C. E.; Afanasjev, A. V.; Austin, R. A. E.; Carpenter, M. P.; Dashdorj, D.; Finlay, P.; Freeman, S. J.; Garrett, P. E.; Greene, J.; Grinyer, G. F.; Görgen, A.; Hyland, B.; Jenkins, D.; Johnston-Theasby, F.; Joshi, P.; Machiavelli, A. O.; Moore, F.; Mukherjee, G.; Phillips, A. A.; Reviol, W.; Sarantites, D. G.; Schumaker, M. A.; Seweryniak, D.; Smith, M. B.; Valiente-Dobón, J. J.; Wadsworth, R.

2007-04-01

High-spin states in the N=Z nucleus Kr72 have been populated in the Ca40(Ca40, 2α)Kr72 fusion-evaporation reaction at a beam energy of 165 MeV using the Gammasphere array for γ-ray detection coupled to the Microball array for charged particle detection. The previously observed bands in Kr72 were extended to an excitation energy of ˜24 MeV and angular momentum of 30ℏ. Using the Doppler shift attenuation method the lifetimes of high-spin states were measured for the first time. Excellent agreement between the results of calculations within the isovector mean field theory and experiment is observed both for rotational and deformation properties. No enhancement of quadrupole deformation expected in the presence of isoscalar t=0 np pairing is observed. Current data do not show any evidence for the existence of the isoscalar np pairing.

EMPIRE: Nuclear Reaction Model Code System for Data Evaluation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Herman, M.; Capote, R.; Carlson, B.V.

EMPIRE is a modular system of nuclear reaction codes, comprising various nuclear models, and designed for calculations over a broad range of energies and incident particles. A projectile can be a neutron, proton, any ion (including heavy-ions) or a photon. The energy range extends from the beginning of the unresolved resonance region for neutron-induced reactions ({approx} keV) and goes up to several hundred MeV for heavy-ion induced reactions. The code accounts for the major nuclear reaction mechanisms, including direct, pre-equilibrium and compound nucleus ones. Direct reactions are described by a generalized optical model (ECIS03) or by the simplified coupled-channels approachmore » (CCFUS). The pre-equilibrium mechanism can be treated by a deformation dependent multi-step direct (ORION + TRISTAN) model, by a NVWY multi-step compound one or by either a pre-equilibrium exciton model with cluster emission (PCROSS) or by another with full angular momentum coupling (DEGAS). Finally, the compound nucleus decay is described by the full featured Hauser-Feshbach model with {gamma}-cascade and width-fluctuations. Advanced treatment of the fission channel takes into account transmission through a multiple-humped fission barrier with absorption in the wells. The fission probability is derived in the WKB approximation within the optical model of fission. Several options for nuclear level densities include the EMPIRE-specific approach, which accounts for the effects of the dynamic deformation of a fast rotating nucleus, the classical Gilbert-Cameron approach and pre-calculated tables obtained with a microscopic model based on HFB single-particle level schemes with collective enhancement. A comprehensive library of input parameters covers nuclear masses, optical model parameters, ground state deformations, discrete levels and decay schemes, level densities, fission barriers, moments of inertia and {gamma}-ray strength functions. The results can be converted into ENDF-6 formatted files using the accompanying code EMPEND and completed with neutron resonances extracted from the existing evaluations. The package contains the full EXFOR (CSISRS) library of experimental reaction data that are automatically retrieved during the calculations. Publication quality graphs can be obtained using the powerful and flexible plotting package ZVView. The graphic user interface, written in Tcl/Tk, provides for easy operation of the system. This paper describes the capabilities of the code, outlines physical models and indicates parameter libraries used by EMPIRE to predict reaction cross sections and spectra, mainly for nucleon-induced reactions. Selected applications of EMPIRE are discussed, the most important being an extensive use of the code in evaluations of neutron reactions for the new US library ENDF/B-VII.0. Future extensions of the system are outlined, including neutron resonance module as well as capabilities of generating covariances, using both KALMAN and Monte-Carlo methods, that are still being advanced and refined.« less

Origins of Singlet Fission in Solid Pentacene from an ab initio Green's Function Approach

NASA Astrophysics Data System (ADS)

Refaely-Abramson, Sivan; da Jornada, Felipe H.; Louie, Steven G.; Neaton, Jeffrey B.

2017-12-01

We develop a new first-principles approach to predict and understand rates of singlet fission with an ab initio Green's-function formalism based on many-body perturbation theory. Starting with singlet and triplet excitons computed from a G W plus Bethe-Salpeter equation approach, we calculate the exciton-biexciton coupling to lowest order in the Coulomb interaction, assuming a final state consisting of two noninteracting spin-correlated triplets with finite center-of-mass momentum. For crystalline pentacene, symmetries dictate that the only purely Coulombic fission decay process from a bright singlet state requires a final state consisting of two inequivalent nearly degenerate triplets of nonzero, equal and opposite, center-of-mass momenta. For such a process, we predict a singlet lifetime of 30-70 fs, in very good agreement with experimental data, indicating that this process can dominate singlet fission in crystalline pentacene. Our approach is general and provides a framework for predicting and understanding multiexciton interactions in solids.

Tidal and Dynamical Evolution of Binary Asteroids

NASA Astrophysics Data System (ADS)

Jacobson, Seth A.; Scheeres, D. J.

2009-05-01

We derive a realistic model for the evolution of a tidally perturbed binary, using classical theory, to examine the system just after a spin-up fission event. The spin rate of an asteroid can be increased by the Yarkovsky-O'Keefe-Radzievskii-Paddack (YORP) effect -- thermal re-radiation from an asymmetric body, which induces torques that can rotationally accelerate the body. If the asteroid is modeled as a "rubble pile", a collection of gravitationally bound gravel with no tensile strength, increasing the spin rate will lead to a fission process that would resemble that of a viscous fluidic body [Holsapple 2007]. However, high-resolution imagery of an asteroid's constituents indicates that there is a significant distribution of size scales. A specific example is the asteroid Itokawa, which appears to be two such rubble piles in contact with each other [Fujiwara 2006]. The shape of these bodies will be irregular (modeled as tri-axial ellipsoids with a gravitational potential expanded up to second order). Their motions will raise tides on the opposing body. These tides will dissipate energy, potentially providing enough energy loss for the system to settle into a stable orbit. Fissioned binary systems are always initially unstable [Scheeres 2009, 2008]. We expect tidal dissipation rates to vary widely during the initial evolution of the system, due to this instability. The model applies instantaneous tidal torques to determine energy loss. Our preliminary results indicate that tidal energy dissipation could relax the system to a state of relative equilibrium on order 100,000 years, creating systems similar to those observed. Holsapple, K. A., Icarus, 187, 2007. Fujiwara, A., Science, 312, 2006. Scheeres, D., CMDA, 2009 (Accepted Jan 10, 2009). Scheeres, D., AAS, DDA meeting #39, #9.01, 2008.

The Explanation of the Pauli Exclusion Principle

NASA Astrophysics Data System (ADS)

Vasiliev, Victor; Moon, Russell

2006-11-01

Using the principles of the Vortex Theory, the construction of the alpha particle, and the theory that the nucleus is constructed out of alpha particles, the explanation of the Pauli Exclusion Principle is explained. If protons and electrons are connected to each other via fourth dimensional vortices, they spin in opposite directions. Since the alpha particle possesses two protons possessing opposite spins, their electrons also possess opposite spins. With a nucleus constructed out of alpha particles, all paired electrons in shells and sub-shells will spin in opposite directions. 1. Victor Vasiliev, Russell Moon. Controversy surrounding the Experiment conducted to prove the Vortex Theory, 2006 8th Annual Meeting of the Northwest Section, May 18-20, 2006, University of Puget Sound, Tacoma, Washington, USA, Abstract C1.00009. 2. Russell Moon. To the Photon Acceleration Effect, 2006 Texas Section APS/AAPT/SPS Joint Spring Meeting, Thursday--Saturday, March 23--25, 2006; San Angelo, Texas, Abstract: POS.00008. 3. Russell Moon, Fabian Calvo, Victor Vasiliev. The Neutral Pentaquark, 2006 APS March Meeting, March 13-17, Baltimore, MD, USA, Session Q1: GENERAL POSTER SESSION, Abstract Q1.00147.

UV photolysis of 4-iodo-, 4-bromo-, and 4-chlorophenol: Competition between C-Y (Y = halogen) and O-H bond fission

NASA Astrophysics Data System (ADS)

Sage, Alan G.; Oliver, Thomas A. A.; King, Graeme A.; Murdock, Daniel; Harvey, Jeremy N.; Ashfold, Michael N. R.

2013-04-01

The wavelength dependences of C-Y and O-H bond fission following ultraviolet photoexcitation of 4-halophenols (4-YPhOH) have been investigated using a combination of velocity map imaging, H Rydberg atom photofragment translational spectroscopy, and high level spin-orbit resolved electronic structure calculations, revealing a systematic evolution in fragmentation behaviour across the series Y = I, Br, Cl (and F). All undergo O-H bond fission following excitation at wavelengths λ ≲ 240 nm, on repulsive ((n/π)σ*) potential energy surfaces (PESs), yielding fast H atoms with mean kinetic energies ˜11 000 cm-1. For Y = I and Br, this process occurs in competition with prompt C-I and C-Br bond cleavage on another (n/π)σ* PES, but no Cl/Cl* products unambiguously attributable to one photon induced C-Cl bond fission are observed from 4-ClPhOH. Differences in fragmentation behaviour at longer excitation wavelengths are more marked. Prompt C-I bond fission is observed following excitation of 4-IPhOH at all λ ≤ 330 nm; the wavelength dependent trends in I/I* product branching ratio, kinetic energy release, and recoil anisotropy suggest that (with regard to C-I bond fission) 4-IPhOH behaves like a mildly perturbed iodobenzene. Br atoms are observed when exciting 4-BrPhOH at long wavelengths also, but their velocity distributions suggest that dissociation occurs after internal conversion to the ground state. O-H bond fission, by tunnelling (as in phenol), is observed only in the cases of 4-FPhOH and, more weakly, 4-ClPhOH. These observed differences in behaviour can be understood given due recognition of (i) the differences in the vertical excitation energies of the C-Y centred (n/π)σ* potentials across the series Y = I < Br < Cl and the concomitant reduction in C-Y bond strength, cf. that of the rival O-H bond, and (ii) the much increased spin-orbit coupling in, particularly, 4-IPhOH. The present results provide (another) reminder of the risks inherent in extrapolating photochemical behaviour measured for one molecule at one wavelength to other (related) molecules and to other excitation energies.

UV photolysis of 4-iodo-, 4-bromo-, and 4-chlorophenol: competition between C-Y (Y = halogen) and O-H bond fission.

PubMed

Sage, Alan G; Oliver, Thomas A A; King, Graeme A; Murdock, Daniel; Harvey, Jeremy N; Ashfold, Michael N R

2013-04-28

The wavelength dependences of C-Y and O-H bond fission following ultraviolet photoexcitation of 4-halophenols (4-YPhOH) have been investigated using a combination of velocity map imaging, H Rydberg atom photofragment translational spectroscopy, and high level spin-orbit resolved electronic structure calculations, revealing a systematic evolution in fragmentation behaviour across the series Y = I, Br, Cl (and F). All undergo O-H bond fission following excitation at wavelengths λ ≲ 240 nm, on repulsive ((n∕π)σ∗) potential energy surfaces (PESs), yielding fast H atoms with mean kinetic energies ∼11,000 cm(-1). For Y = I and Br, this process occurs in competition with prompt C-I and C-Br bond cleavage on another (n∕π)σ∗ PES, but no Cl∕Cl∗ products unambiguously attributable to one photon induced C-Cl bond fission are observed from 4-ClPhOH. Differences in fragmentation behaviour at longer excitation wavelengths are more marked. Prompt C-I bond fission is observed following excitation of 4-IPhOH at all λ ≤ 330 nm; the wavelength dependent trends in I∕I∗ product branching ratio, kinetic energy release, and recoil anisotropy suggest that (with regard to C-I bond fission) 4-IPhOH behaves like a mildly perturbed iodobenzene. Br atoms are observed when exciting 4-BrPhOH at long wavelengths also, but their velocity distributions suggest that dissociation occurs after internal conversion to the ground state. O-H bond fission, by tunnelling (as in phenol), is observed only in the cases of 4-FPhOH and, more weakly, 4-ClPhOH. These observed differences in behaviour can be understood given due recognition of (i) the differences in the vertical excitation energies of the C-Y centred (n∕π)σ∗ potentials across the series Y = I < Br < Cl and the concomitant reduction in C-Y bond strength, cf. that of the rival O-H bond, and (ii) the much increased spin-orbit coupling in, particularly, 4-IPhOH. The present results provide (another) reminder of the risks inherent in extrapolating photochemical behaviour measured for one molecule at one wavelength to other (related) molecules and to other excitation energies.

On The Geometric Nature of ``Singlet Fission'' in Certain Crystalline Conjugated Polymers

NASA Astrophysics Data System (ADS)

Rahman, Noah

2013-03-01

In recent years, the coherent fission of low-lying singlet electronic excitations in conjugated polymers has attracted interest as a possible way to exceed the Shockley-Queisser limit in organic photovoltaics. Femtosecond spectroscopic and fluorescence measurements of such singlets and the resulting triplets in crystalline anthracene, tetracene and naphthalene reveal curious phenomena associated with certain vibrational modes, such as ultrafast propagation on a timescale inconsistent with conventional intersystem crossing, long-lived electronic coherence, and triplet magnetic anisotropy whose structure is consistent across all three materials. This conflicts with NRG and quantum chemical simulations, which posit isotropic triplets. I explain this by a dynamical Rashba spin-orbit interaction that decays as R-6. This arises from a geometric SU(2) gauge potential generated by a nuclear-motion-induced parametric near-degeneracy of the molecular electronic states. The anisotropy is shown to follow from the work of Affleck and Oshikawa on spin one-half Heisenberg chains. Possible directions for future work are discussed, especially with regard to adiabatic pumping and topological insulators.

Precision Measurement of the β Asymmetry in Spin-Polarized K 37 Decay

NASA Astrophysics Data System (ADS)

Fenker, B.; Gorelov, A.; Melconian, D.; Behr, J. A.; Anholm, M.; Ashery, D.; Behling, R. S.; Cohen, I.; Craiciu, I.; Gwinner, G.; McNeil, J.; Mehlman, M.; Olchanski, K.; Shidling, P. D.; Smale, S.; Warner, C. L.

2018-02-01

Using Triumf's neutral atom trap, Trinat, for nuclear β decay, we have measured the β asymmetry with respect to the initial nuclear spin in K 37 to be Aβ=-0.5707 (13) syst(13) stat(5) pol , a 0.3% measurement. This is the best relative accuracy of any β -asymmetry measurement in a nucleus or the neutron, and is in agreement with the standard model prediction -0.5706 (7 ). We compare constraints on physics beyond the standard model with other β -decay measurements, and improve the value of Vud measured in this mirror nucleus by a factor of 4.

Microscopic theory of nuclear fission: a review

NASA Astrophysics Data System (ADS)

Schunck, N.; Robledo, L. M.

2016-11-01

This article reviews how nuclear fission is described within nuclear density functional theory. A distinction should be made between spontaneous fission, where half-lives are the main observables and quantum tunnelling the essential concept, and induced fission, where the focus is on fragment properties and explicitly time-dependent approaches are often invoked. Overall, the cornerstone of the density functional theory approach to fission is the energy density functional formalism. The basic tenets of this method, including some well-known tools such as the Hartree-Fock-Bogoliubov (HFB) theory, effective two-body nuclear potentials such as the Skyrme and Gogny force, finite-temperature extensions and beyond mean-field corrections, are presented succinctly. The energy density functional approach is often combined with the hypothesis that the time-scale of the large amplitude collective motion driving the system to fission is slow compared to typical time-scales of nucleons inside the nucleus. In practice, this hypothesis of adiabaticity is implemented by introducing (a few) collective variables and mapping out the many-body Schrödinger equation into a collective Schrödinger-like equation for the nuclear wave-packet. The region of the collective space where the system transitions from one nucleus to two (or more) fragments defines what are called the scission configurations. The inertia tensor that enters the kinetic energy term of the collective Schrödinger-like equation is one of the most essential ingredients of the theory, since it includes the response of the system to small changes in the collective variables. For this reason, the two main approximations used to compute this inertia tensor, the adiabatic time-dependent HFB and the generator coordinate method, are presented in detail, both in their general formulation and in their most common approximations. The collective inertia tensor enters also the Wentzel-Kramers-Brillouin (WKB) formula used to extract spontaneous fission half-lives from multi-dimensional quantum tunnelling probabilities (For the sake of completeness, other approaches to tunnelling based on functional integrals are also briefly discussed, although there are very few applications.) It is also an important component of some of the time-dependent methods that have been used in fission studies. Concerning the latter, both the semi-classical approaches to time-dependent nuclear dynamics and more microscopic theories involving explicit quantum-many-body methods are presented. One of the hallmarks of the microscopic theory of fission is the tremendous amount of computing needed for practical applications. In particular, the successful implementation of the theories presented in this article requires a very precise numerical resolution of the HFB equations for large values of the collective variables. This aspect is often overlooked, and several sections are devoted to discussing the resolution of the HFB equations, especially in the context of very deformed nuclear shapes. In particular, the numerical precision and iterative methods employed to obtain the HFB solution are documented in detail. Finally, a selection of the most recent and representative results obtained for both spontaneous and induced fission is presented, with the goal of emphasizing the coherence of the microscopic approaches employed. Although impressive progress has been achieved over the last two decades to understand fission microscopically, much work remains to be done. Several possible lines of research are outlined in the conclusion.

Microscopic Theory of Nuclear Fission: A Review

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schunck, N.; Robledo, L. M.

This paper reviews how nuclear fission is described within nuclear density functional theory. A distinction should be made between spontaneous fission, where half-lives are the main observables and quantum tunnelling the essential concept, and induced fission, where the focus is on fragment properties and explicitly time-dependent approaches are often invoked. Overall, the cornerstone of the density functional theory approach to fission is the energy density functional formalism. The basic tenets of this method, including some well-known tools such as the Hartree–Fock–Bogoliubov (HFB) theory, effective two-body nuclear potentials such as the Skyrme and Gogny force, finite-temperature extensions and beyond mean-field corrections,more » are presented succinctly. The energy density functional approach is often combined with the hypothesis that the time-scale of the large amplitude collective motion driving the system to fission is slow compared to typical time-scales of nucleons inside the nucleus. In practice, this hypothesis of adiabaticity is implemented by introducing (a few) collective variables and mapping out the many-body Schrödinger equation into a collective Schrödinger-like equation for the nuclear wave-packet. The region of the collective space where the system transitions from one nucleus to two (or more) fragments defines what are called the scission configurations. The inertia tensor that enters the kinetic energy term of the collective Schrödinger-like equation is one of the most essential ingredients of the theory, since it includes the response of the system to small changes in the collective variables. For this reason, the two main approximations used to compute this inertia tensor, the adiabatic time-dependent HFB and the generator coordinate method, are presented in detail, both in their general formulation and in their most common approximations. The collective inertia tensor enters also the Wentzel–Kramers–Brillouin (WKB) formula used to extract spontaneous fission half-lives from multi-dimensional quantum tunnelling probabilities (For the sake of completeness, other approaches to tunnelling based on functional integrals are also briefly discussed, although there are very few applications.) It is also an important component of some of the time-dependent methods that have been used in fission studies. Concerning the latter, both the semi-classical approaches to time-dependent nuclear dynamics and more microscopic theories involving explicit quantum-many-body methods are presented. One of the hallmarks of the microscopic theory of fission is the tremendous amount of computing needed for practical applications. In particular, the successful implementation of the theories presented in this article requires a very precise numerical resolution of the HFB equations for large values of the collective variables. This aspect is often overlooked, and several sections are devoted to discussing the resolution of the HFB equations, especially in the context of very deformed nuclear shapes. In particular, the numerical precision and iterative methods employed to obtain the HFB solution are documented in detail. Finally, a selection of the most recent and representative results obtained for both spontaneous and induced fission is presented, with the goal of emphasizing the coherence of the microscopic approaches employed. In conclusion, although impressive progress has been achieved over the last two decades to understand fission microscopically, much work remains to be done. Several possible lines of research are outlined in the conclusion.« less

Microscopic Theory of Nuclear Fission: A Review

DOE PAGES

Schunck, N.; Robledo, L. M.

2016-10-11

This paper reviews how nuclear fission is described within nuclear density functional theory. A distinction should be made between spontaneous fission, where half-lives are the main observables and quantum tunnelling the essential concept, and induced fission, where the focus is on fragment properties and explicitly time-dependent approaches are often invoked. Overall, the cornerstone of the density functional theory approach to fission is the energy density functional formalism. The basic tenets of this method, including some well-known tools such as the Hartree–Fock–Bogoliubov (HFB) theory, effective two-body nuclear potentials such as the Skyrme and Gogny force, finite-temperature extensions and beyond mean-field corrections,more » are presented succinctly. The energy density functional approach is often combined with the hypothesis that the time-scale of the large amplitude collective motion driving the system to fission is slow compared to typical time-scales of nucleons inside the nucleus. In practice, this hypothesis of adiabaticity is implemented by introducing (a few) collective variables and mapping out the many-body Schrödinger equation into a collective Schrödinger-like equation for the nuclear wave-packet. The region of the collective space where the system transitions from one nucleus to two (or more) fragments defines what are called the scission configurations. The inertia tensor that enters the kinetic energy term of the collective Schrödinger-like equation is one of the most essential ingredients of the theory, since it includes the response of the system to small changes in the collective variables. For this reason, the two main approximations used to compute this inertia tensor, the adiabatic time-dependent HFB and the generator coordinate method, are presented in detail, both in their general formulation and in their most common approximations. The collective inertia tensor enters also the Wentzel–Kramers–Brillouin (WKB) formula used to extract spontaneous fission half-lives from multi-dimensional quantum tunnelling probabilities (For the sake of completeness, other approaches to tunnelling based on functional integrals are also briefly discussed, although there are very few applications.) It is also an important component of some of the time-dependent methods that have been used in fission studies. Concerning the latter, both the semi-classical approaches to time-dependent nuclear dynamics and more microscopic theories involving explicit quantum-many-body methods are presented. One of the hallmarks of the microscopic theory of fission is the tremendous amount of computing needed for practical applications. In particular, the successful implementation of the theories presented in this article requires a very precise numerical resolution of the HFB equations for large values of the collective variables. This aspect is often overlooked, and several sections are devoted to discussing the resolution of the HFB equations, especially in the context of very deformed nuclear shapes. In particular, the numerical precision and iterative methods employed to obtain the HFB solution are documented in detail. Finally, a selection of the most recent and representative results obtained for both spontaneous and induced fission is presented, with the goal of emphasizing the coherence of the microscopic approaches employed. In conclusion, although impressive progress has been achieved over the last two decades to understand fission microscopically, much work remains to be done. Several possible lines of research are outlined in the conclusion.« less

Microscopic theory of nuclear fission: a review.

PubMed

Schunck, N; Robledo, L M

2016-11-01

This article reviews how nuclear fission is described within nuclear density functional theory. A distinction should be made between spontaneous fission, where half-lives are the main observables and quantum tunnelling the essential concept, and induced fission, where the focus is on fragment properties and explicitly time-dependent approaches are often invoked. Overall, the cornerstone of the density functional theory approach to fission is the energy density functional formalism. The basic tenets of this method, including some well-known tools such as the Hartree-Fock-Bogoliubov (HFB) theory, effective two-body nuclear potentials such as the Skyrme and Gogny force, finite-temperature extensions and beyond mean-field corrections, are presented succinctly. The energy density functional approach is often combined with the hypothesis that the time-scale of the large amplitude collective motion driving the system to fission is slow compared to typical time-scales of nucleons inside the nucleus. In practice, this hypothesis of adiabaticity is implemented by introducing (a few) collective variables and mapping out the many-body Schrödinger equation into a collective Schrödinger-like equation for the nuclear wave-packet. The region of the collective space where the system transitions from one nucleus to two (or more) fragments defines what are called the scission configurations. The inertia tensor that enters the kinetic energy term of the collective Schrödinger-like equation is one of the most essential ingredients of the theory, since it includes the response of the system to small changes in the collective variables. For this reason, the two main approximations used to compute this inertia tensor, the adiabatic time-dependent HFB and the generator coordinate method, are presented in detail, both in their general formulation and in their most common approximations. The collective inertia tensor enters also the Wentzel-Kramers-Brillouin (WKB) formula used to extract spontaneous fission half-lives from multi-dimensional quantum tunnelling probabilities (For the sake of completeness, other approaches to tunnelling based on functional integrals are also briefly discussed, although there are very few applications.) It is also an important component of some of the time-dependent methods that have been used in fission studies. Concerning the latter, both the semi-classical approaches to time-dependent nuclear dynamics and more microscopic theories involving explicit quantum-many-body methods are presented. One of the hallmarks of the microscopic theory of fission is the tremendous amount of computing needed for practical applications. In particular, the successful implementation of the theories presented in this article requires a very precise numerical resolution of the HFB equations for large values of the collective variables. This aspect is often overlooked, and several sections are devoted to discussing the resolution of the HFB equations, especially in the context of very deformed nuclear shapes. In particular, the numerical precision and iterative methods employed to obtain the HFB solution are documented in detail. Finally, a selection of the most recent and representative results obtained for both spontaneous and induced fission is presented, with the goal of emphasizing the coherence of the microscopic approaches employed. Although impressive progress has been achieved over the last two decades to understand fission microscopically, much work remains to be done. Several possible lines of research are outlined in the conclusion.

Studying fission neutrons with 2E-2v and 2E

NASA Astrophysics Data System (ADS)

Al-Adili, Ali; Jansson, Kaj; Tarrío, Diego; Hambsch, Franz-Josef; Göök, Alf; Oberstedt, Stephan; Olivier Frégeau, Marc; Gustavsson, Cecilia; Lantz, Mattias; Mattera, Andrea; Prokofiev, Alexander V.; Rakopoulos, Vasileios; Solders, Andreas; Vidali, Marzio; Österlund, Michael; Pomp, Stephan

2018-03-01

This work aims at measuring prompt-fission neutrons at different excitation energies of the nucleus. Two independent techniques, the 2E-2v and the 2E techniques, are used to map the characteristics of the mass-dependent prompt fission neutron multiplicity, v(A), when the excitation energy is increased. The VERDI 2E-2v spectrometer is being developed at JRC-GEEL. The Fission Fragment (FF) energies are measured using two arrays of 16 silicon (Si) detectors each. The FFs velocities are obtained by time-of-flight, measured between micro-channel plates (MCP) and Si detectors. With MCPs placed on both sides of the fission source, VERDI allows for independent timing measurements for both fragments. 252Cf(sf) was measured and the present results revealed particular features of the 2E-2v technique. Dedicated simulations were also performed using the GEF code to study important aspects of the 2E-2v technique. Our simulations show that prompt neutron emission has a non-negligible impact on the deduced fragment data and affects also the shape of v(A). Geometrical constraints lead to a total-kinetic energy-dependent detection efficiency. The 2E technique utilizes an ionization chamber together with two liquid scintillator detectors. Two measurements have been performed, one of 252Cf(sf) and another one of thermal-neutron induced fission in 235U(n,f). Results from 252Cf(sf) are reported here.

Tuning Singlet Fission in π-Bridge-π Chromophores

DOE PAGES

Kumarasamy, Elango; Sanders, Samuel N.; Tayebjee, Murad J. Y.; ...

2017-08-11

For this study, we have designed a series of pentacene dimers separated by homoconjugated or nonconjugated bridges that exhibit fast and efficient intramolecular singlet exciton fission (iSF). These materials are distinctive among reported iSF compounds because they exist in the unexplored regime of close spatial proximity but weak electronic coupling between the singlet exciton and triplet pair states. Using transient absorption spectroscopy to investigate photophysics in these molecules, we find that homoconjugated dimers display desirable excited-state dynamics, with significantly reduced recombination rates as compared to conjugated dimers with similar singlet fission rates. In addition, unlike conjugated dimers, the time constantsmore » for singlet fission are relatively insensitive to the interplanar angle between chromophores, since rotation about σ bonds negligibly affects the orbital overlap within the π-bonding network. In the nonconjugated dimer, where the iSF occurs with a time constant >10 ns, comparable to the fluorescence lifetime, we used electron spin resonance spectroscopy to unequivocally establish the formation of triplet–triplet multiexcitons and uncoupled triplet excitons through singlet fission. Together, these studies enable us to articulate the role of the conjugation motif in iSF.« less

Forced precession of the cometary nucleus with randomly placed active regions

NASA Technical Reports Server (NTRS)

Szutowicz, Slawomira

1992-01-01

The cometary nucleus is assumed to be triaxial or axisymmetric spheroid rotating about its axis of maximum moment of inertia and is forced to precess due to jets of ejected material. Randomly placed regions of exposed ice on the surface of the nucleus are assumed to produce gas and dust. The solution of the heat conduction equation for each active region is used to find the gas sublimation rate and the jet acceleration. Precession of the comet nucleus is followed numerically using a phase-averaged system of equations. The gas production curves and the variation of the spin axis during the orbital motion of the comet are presented.

Improvement of gross theory of beta-decay for application to nuclear data

NASA Astrophysics Data System (ADS)

Koura, Hiroyuki; Yoshida, Tadashi; Tachibana, Takahiro; Chiba, Satoshi

2017-09-01

A theoretical study of β decay and delayed neutron has been carried out with a global β-decay model, the gross theory. The gross theory is based on a consideration of the sum rule of the β-strength function, and gives reasonable results of β-decay rates and delayed neutron in the entire nuclear mass region. In a fissioning nucleus, neutrons are produced by β decay of neutron-rich fission fragments from actinides known as delayed neutrons. The average number of delayed neutrons is estimated based on the sum of the β-delayed neutron-emission probabilities multiplied by the cumulative fission yield for each nucleus. Such a behavior is important to manipulate nuclear reactors, and when we adopt some new high-burn-up reactors, properties of minor actinides will play an important roll in the system, but these data have not been sufficient. We re-analyze and improve the gross theory. For example, we considered the parity of neutrons and protons at the Fermi surface, and treat a suppression for the allowed transitions in the framework of the gross theory. By using the improved gross theory, underestimated half-lives in the neutron-rich indium isotopes and neighboring region increase, and consequently follow experimental trend. The ability of reproduction (and also prediction) of the β-decay rates, delayed-neutron emission probabilities is discussed. With this work, we have described the development of a programming code of the gross theory of β-decay including the improved parts. After preparation finished, this code can be released for the nuclear data community.

Evaluation of the 235U prompt fission neutron spectrum including a detailed analysis of experimental data and improved model information

DOE Office of Scientific and Technical Information (OSTI.GOV)

Neudecker, Denise; Talou, Patrick; Kahler, Albert Comstock III

We present an evaluation of the 235U prompt fission neutron spectrum (PFNS) induced by thermal to 20-MeV neutrons. Experimental data and associated covariances were analyzed in detail. The incident energy dependence of the PFNS was modeled with an extended Los Alamos model combined with the Hauser-Feshbach and the exciton models. These models describe prompt fission, pre-fission compound nucleus and pre-equilibrium neutron emissions. The evaluated PFNS agree well with the experimental data included in this evaluation, preliminary data of the LANL and LLNL Chi-Nu measurement and recent evaluations by Capote et al. and Rising et al. However, they are softer thanmore » the ENDF/B-VII.1 (VII.1) and JENDL-4.0 PFNS for incident neutron energies up to 2 MeV. Simulated effective multiplication factors k eff of the Godiva and Flattop-25 critical assemblies are further from the measured k eff if the current data are used within VII.1 compared to using only VII.1 data. However, if this work is used with ENDF/B-VIII.0β2 data, simulated values of k eff agree well with the measured ones.« less

Evaluation of the 235U prompt fission neutron spectrum including a detailed analysis of experimental data and improved model information

DOE PAGES

Neudecker, Denise; Talou, Patrick; Kahler, Albert Comstock III; ...

2017-09-13

We present an evaluation of the 235U prompt fission neutron spectrum (PFNS) induced by thermal to 20-MeV neutrons. Experimental data and associated covariances were analyzed in detail. The incident energy dependence of the PFNS was modeled with an extended Los Alamos model combined with the Hauser-Feshbach and the exciton models. These models describe prompt fission, pre-fission compound nucleus and pre-equilibrium neutron emissions. The evaluated PFNS agree well with the experimental data included in this evaluation, preliminary data of the LANL and LLNL Chi-Nu measurement and recent evaluations by Capote et al. and Rising et al. However, they are softer thanmore » the ENDF/B-VII.1 (VII.1) and JENDL-4.0 PFNS for incident neutron energies up to 2 MeV. Simulated effective multiplication factors k eff of the Godiva and Flattop-25 critical assemblies are further from the measured k eff if the current data are used within VII.1 compared to using only VII.1 data. However, if this work is used with ENDF/B-VIII.0β2 data, simulated values of k eff agree well with the measured ones.« less

Search for ternary fission of chromium-48

NASA Astrophysics Data System (ADS)

Dummer, Andrew K.

1999-07-01

Both alpha cluster model calculations and macroscopic energy calculations that allow for a double-neck shape of the compound nucleus suggest the possibility of a novel three 16O, chain-like configuration in 48 Cr. Such a configuration might lead to an enhanced cross section for three-16O breakup. To explore this possibility, the three-body exit channels for the 36Ar + 12C reaction at a beam energy of 210 MeV have been studied. The cross section for 16O + 16O + 16O breakup has been deduced and has been found to be in excess of what would be expected to result from a sequential binary fission process. However, the observation of a similarly enhanced 12C + 16O + 20Ne breakup cross section suggests that the observed 16O + 16O + 16O yields might still be associated with a statistical fission process. The results are discussed in the context of the fission of light nuclear systems and a simple cluster model calculation. This latter, ``Harvey model'' calculation suggests a possible inhibition of the formation of a three- 16O chain configuration from the 36Ar + 12C entrance channel. A further measurement using the 20Ne + 28Si-entrance channel is suggested.

Evaluation of the 235U prompt fission neutron spectrum including a detailed analysis of experimental data and improved model information

NASA Astrophysics Data System (ADS)

Neudecker, Denise; Talou, Patrick; Kahler, Albert C.; White, Morgan C.; Kawano, Toshihiko

2017-09-01

We present an evaluation of the 235U prompt fission neutron spectrum (PFNS) induced by thermal to 20-MeV neutrons. Experimental data and associated covariances were analyzed in detail. The incident energy dependence of the PFNS was modeled with an extended Los Alamos model combined with the Hauser-Feshbach and the exciton models. These models describe prompt fission, pre-fission compound nucleus and pre-equilibrium neutron emissions. The evaluated PFNS agree well with the experimental data included in this evaluation, preliminary data of the LANL and LLNL Chi-Nu measurement and recent evaluations by Capote et al. and Rising et al. However, they are softer than the ENDF/B-VII.1 (VII.1) and JENDL-4.0 PFNS for incident neutron energies up to 2 MeV. Simulated effective multiplication factors keff of the Godiva and Flattop-25 critical assemblies are further from the measured keff if the current data are used within VII.1 compared to using only VII.1 data. However, if this work is used with ENDF/B-VIII.0β2 data, simulated values of keff agree well with the measured ones.

On the dust zoning of rapidly rotating cometary nuclei

NASA Astrophysics Data System (ADS)

Houpis, H. L. F.; Mendis, D. A.

1981-12-01

The effects of nuclear rotation on the surface of a cometary nucleus (a comet at 1 AU that is H2O dominated and has a radius of 1 km) are considered. It is shown that this dust does not accumulate uniformly on the surface, which here is considered spherical. While dust particles in the two polar cap regions and an equatorial belt remain at rest on the surface, those in two midlatitude bands migrate toward the equator, stopping at the two low latitudes to form dust ridges. As the nucleus spins up, both the polar caps and the equatorial belt shrink in size, and the dust ridges move toward the equator, eventually spinning off the dust from the nucleus when the nuclear rotation period is less than about 3.3 hr. For larger particles for which the gas buoyancy is negligible, migration takes place only if the rotation period is not significantly larger than the critical value of 3.3 hr or if the surface friction is abnormally small.

New observations and new models of spin-orbit coupling in binary asteroids

NASA Astrophysics Data System (ADS)

Margot, Jean-Luc; Naidu, Shantanu

2015-08-01

The YORP-induced rotational fission hypothesis is the leading candidate for explaining the formation of binaries, triples, and pairs among small (<20 km) asteroids (e.g., Margot et al, Asteroids IV, subm., 2015). Various evolutionary paths following rotational fission have been suggested, but many important questions remain about the evolutionary mechanisms and timescales. We test hypotheses about the evolution of binary asteroids by obtaining precise descriptions of the orbits and components of binary systems with radar and by examining the system dynamics with detailed numerical simulations. Predictions for component spin states and orbital precession rates can then be compared to observables in our data sets or in other data sets to elucidate the states of various systems and their likely evolutionary paths.Accurate simulations require knowledge of the masses, shapes, and spin states of individual binary components. Because radar observations can provide exquisite data sets spanning days with spatial resolutions at the decameter level, we can invert for the component shapes and measure spin states. We can also solve for the mutual orbit by fitting the observed separations between components. In addition, the superb (10e-7--10e-8) fractional uncertainties in range allow us to measure the reflex motions directly, allowing masses of individual components to be determined.We use recently published observations of the binary 2000 DP107 (Naidu et al. AJ, subm., 2015) and that of other systems to simulate the dynamics of components in well-characterized binary systems (Naidu and Margot, AJ 149, 80, 2015). We model the coupled spin and orbital motions of two rigid, ellipsoidal bodies under the influence of their mutual gravitational potential. We use surface of section plots to map the possible spin configurations of the satellites. For asynchronous satellites, the analysis reveals large regions of phase space where the spin state of the satellite is chaotic. The presence of chaotic regions may substantially increase spin synchronization timescales, delay BYORP-type evolution, extend the lifetime of binaries, and explain the observed fraction of asynchronous binaries.

Nucleus model for periodic Comet Tempel 2

NASA Technical Reports Server (NTRS)

Sekanina, Zdenek

1991-01-01

Observational data obtained primarily during 1988 are analyzed and synthesized to develop a comprehensive physical model for the nucleus of Periodic Comet Tempel 2, one of the best studied members of Jupiter's family of short-period comets. It is confirmed that a previous investigation provided reliable information on the comet's spin-axis orientation, which implies and obliquity of 54 degrees of the orbit plane to the equatorial plane and which appears to have varied little - if at all - with time. This conclusion is critical for fitting a triaxial ellipsoid to approximate the figure of the nucleus.

Is Einstein the Father of the Atomic Bomb

NASA Astrophysics Data System (ADS)

Lustig, Harry

2009-05-01

Soon after the American atomic bombs were dropped on Hiroshima and Nagasaki, the notion took hold in the popular mind that Albert Einstein was ``the father of the bomb.'' The claim of paternity rests on the belief that E=mc2 is what makes the release of enormous amounts of energy in the fission process possible and that the atomic bomb could not have been built without it. This is a misapprehension. Most physicists have known that all along. Nevertheless in his reaction to the opera Dr. Atomic, a prominent physicist claimed that Einstein's discovery that matter can be transformed into energy ``is precisely what made the bomb possible.'' In fact what makes the fission reaction and one of its applications,the atomic bomb, possible is the smaller binding energies of fission products compared to the binding energies of the nuclei that undergo fission.The binding energies of nuclei are a well understood consequence of the numbers and arrangements of protons and neutrons in the nucleus and of quantum-mechanical effects. The realization that composite systems have binding energies predates relativity. In the 19th century they were ascribed to potential and other forms of energy that reside in the system. With Einstein they became rest mass energy. While E=mc2 is not the cause of fission, measuring the masses of the participants in the reaction does permit an easy calculation of the kinetic energy that is released.

Computer studies of multiple-quantum spin dynamics

DOE Office of Scientific and Technical Information (OSTI.GOV)

Murdoch, J.B.

The excitation and detection of multiple-quantum (MQ) transitions in Fourier transform NMR spectroscopy is an interesting problem in the quantum mechanical dynamics of spin systems as well as an important new technique for investigation of molecular structure. In particular, multiple-quantum spectroscopy can be used to simplify overly complex spectra or to separate the various interactions between a nucleus and its environment. The emphasis of this work is on computer simulation of spin-system evolution to better relate theory and experiment.

Fast passage dynamic nuclear polarization on rotating solids

NASA Astrophysics Data System (ADS)

Mentink-Vigier, Frederic; Akbey, Ümit; Hovav, Yonatan; Vega, Shimon; Oschkinat, Hartmut; Feintuch, Akiva

2012-11-01

Magic Angle Spinning (MAS) Dynamic Nuclear Polarization (DNP) has proven to be a very powerful way to improve the signal to noise ratio of NMR experiments on solids. The experiments have in general been interpreted considering the Solid-Effect (SE) and Cross-Effect (CE) DNP mechanisms while ignoring the influence of sample spinning. In this paper, we show experimental data of MAS-DNP enhancements of 1H and 13C in proline and SH3 protein in glass forming water/glycerol solvent containing TOTAPOL. We also introduce a theoretical model that aims at explaining how the nuclear polarization is built in MAS-DNP experiments. By using Liouville space based simulations to include relaxation on two simple spin models, {electron-nucleus} and {electron-electron-nucleus}, we explain how the basic MAS-SE-DNP and MAS-CE-DNP processes work. The importance of fast energy passages and short level anti-crossing is emphasized and the differences between static DNP and MAS-DNP is explained. During a single rotor cycle the enhancement in the {electron-electron-nucleus} system arises from MAS-CE-DNP involving at least three kinds of two-level fast passages: an electron-electron dipolar anti-crossing, a single quantum electron MW encounter and an anti-crossing at the CE condition inducing nuclear polarization in- or decrements. Numerical, powder-averaged, simulations were performed in order to check the influence of the experimental parameters on the enhancement efficiencies. In particular we show that the spinning frequency dependence of the theoretical MAS-CE-DNP enhancement compares favorably with the experimental 1H and 13C MAS-DNP enhancements of proline and SH3.

Spin differences in the Zr 90 compound nucleus induced by ( p , p ' ) , ( p , d ) , and ( p , t ) surrogate reactions

DOE PAGES

Ota, S.; Burke, J. T.; Casperson, R. J.; ...

2015-11-04

Here, the effect of the production mechanism on the decay of a compound nucleus is investigated. The nucleus 90Zr was produced by three different reactions, namely 90Zr (p,p') 90Zr, 91Zr (p,d) 90Zr, and 92Zr (p,t) 90Zr , which served as surrogate reactions for 89Zr (n,γ). The spin-parity (J π) distributions of the states populated by these reactions were studied to investigate the surrogate reaction approach, which aims at indirectly determining cross sections for compound-nuclear reactions involving unstable targets such as 89Zr. Discrete γ rays, associated with transitions in 90Zr and 89Zr, were measured in coincidence with light ions for scatteringmore » angles of 25°–60° and 90Zr excitation energies extending above the neutron separation energy. The measured transition systematics were used to gain insights into the J π distributions of 90Zr. The 90Zr (p,p') reaction was found to produce fewer γ rays associated with transitions involving high spin states (J = 6–8 ℏ) than the other two reactions, suggesting that inelastic scattering preferentially populates states in 90Zr that have lower spins than those populated in the transfer reactions investigated. The γ-ray production was also observed to vary by factors of 2–3 with the angle at which the outgoing particle was detected. These findings are relevant to the application of the surrogate reaction approach.« less

Spectroscopy of the odd-odd fp-shell nucleus {sup 52}Sc from secondary fragmentation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gade, A.; Bazin, D.; Mueller, W.F.

2006-03-15

The odd-odd fp-shell nucleus {sup 52}Sc was investigated using in-beam {gamma}-ray spectroscopy following secondary fragmentation of a {sup 55}V and {sup 57}Cr cocktail beam. Aside from the known {gamma}-ray transition at 674(5) keV, a new decay at E{sub {gamma}}=212(3) keV was observed. It is attributed to the depopulation of a low-lying excited level. This new state is discussed in the framework of shell-model calculations with the GXPF1, GXPF1A, and KB3G effective interactions. These calculations are found to be fairly robust for the low-lying level scheme of {sup 52}Sc irrespective of the choice of the effective interaction. In addition, the frequencymore » of spin values predicted by the shell model is successfully modeled by a spin distribution formulated in a statistical approach with an empirical, energy-independent spin-cutoff parameter.« less

Fission Fragment Studies by Gamma-Ray Spectrometry with the Mass Separator Lohengrin

NASA Astrophysics Data System (ADS)

Materna, T.; Amouroux, C.; Bail, A.; Bideau, A.; Chabod, S.; Faust, H.; Capellan, N.; Kessedjian, G.; Köster, U.; Letourneau, A.; Litaize, O.; Martin, F.; Mathieu, L.; Méplan, O.; Panebianco, S.; Régis, J.-M.; Rudigier, M.; Sage, C.; Serot, O.; Urban, W.

2014-09-01

A gamma spectrometric technique was implemented at the exit of the fission fragment separator of the ILL. It allows a precise measurement of isotopic yields of most important actinides in the heavy fragment region by an unambiguous identification of the nuclear charge of the fragments selected by the mass spectrometer. The status of the project and last results are reviewed. A spin-off of this activity is the identification of unknown nanosecond isomers in exotic nuclei through the observation of a disturbed ionic charge distribution. This technique has been improved to provide an estimation of the lifetime of the isomeric state.

Recoil- α -fission and recoil- α – α -fission events observed in the reaction 48 Ca + 243 Am

DOE PAGES

Forsberg, U.; Rudolph, D.; Andersson, L. -L.; ...

2016-04-26

A recent high-resolution α, X-ray, and γ-ray coincidence-spectroscopy experiment at GSI offered the first glimpse of excitation schemes of isotopes along α-decay chains of Z=115. To understand these observations and to make predictions about shell structure of superheavy nuclei below 288115, we employed nuclear DFT. We find that the presence and nature of low-energy E1 transitions in well-deformed nuclei around Z=110, N=168 strongly depends on the strength of the spin-orbit coupling; hence, it provides an excellent constraint on theoretical models of superheavy nuclei.

Cobalt spin states and hyperfine interactions in LaCoO3 investigated by LDA+U calculations

NASA Astrophysics Data System (ADS)

Hsu, Han; Blaha, Peter; Wentzcovitch, Renata M.; Leighton, C.

2010-09-01

With a series of local-density approximation plus Hubbard U calculations, we have demonstrated that for lanthanum cobaltite (LaCoO3) , the electric field gradient at the cobalt nucleus can be used as a fingerprint to identify the spin state of the cobalt ion. Therefore, in principle, the spin state of the cobalt ion can be unambiguously determined from nuclear magnetic resonance spectra. Our calculations also suggest that a crossover from the low-spin to intermediate-spin state in the temperature range of 0-90 K is unlikely, based on the half-metallic band structure associated with isolated IS Co ions, which is incompatible with the measured conductivity.

Benchmarking singlet and triplet excitation energies of molecular semiconductors for singlet fission: Tuning the amount of HF exchange and adjusting local correlation to obtain accurate functionals for singlet-triplet gaps

NASA Astrophysics Data System (ADS)

Brückner, Charlotte; Engels, Bernd

2017-01-01

Vertical and adiabatic singlet and triplet excitation energies of molecular p-type semiconductors calculated with various DFT functionals and wave-function based approaches are benchmarked against MS-CASPT2/cc-pVTZ reference values. A special focus lies on the singlet-triplet gaps that are very important in the process of singlet fission. Singlet fission has the potential to boost device efficiencies of organic solar cells, but the scope of existing singlet-fission compounds is still limited. A computational prescreening of candidate molecules could enlarge it; yet it requires efficient methods accurately predicting singlet and triplet excitation energies. Different DFT formulations (Tamm-Dancoff approximation, linear response time-dependent DFT, Δ-SCF) and spin scaling schemes along with several ab initio methods (CC2, ADC(2)/MP2, CIS(D), CIS) are evaluated. While wave-function based methods yield rather reliable singlet-triplet gaps, many DFT functionals are shown to systematically underestimate triplet excitation energies. To gain insight, the impact of exact exchange and correlation is in detail addressed.

The pure rotational spectrum of TiF (X 4Φr): 3d transition metal fluorides revisited

NASA Astrophysics Data System (ADS)

Sheridan, P. M.; McLamarrah, S. K.; Ziurys, L. M.

2003-11-01

The pure rotational spectrum of TiF in its X 4Φr (v=0) ground state has been measured using millimeter/sub-millimeter wave direct absorption techniques in the range 140-530 GHz. In ten out of the twelve rotational transitions recorded, all four spin-orbit components were observed, confirming the 4Φr ground state assignment. Additional small splittings were resolved in several of the spin components in lower J transitions, which appear to arise from magnetic hyperfine interactions of the 19F nucleus. In contrast, no evidence for Λ-doubling was seen in the data. The rotational transitions of TiF were analyzed using a case (a) Hamiltonian, resulting in the determination of rotational and fine structure constants, as well as hyperfine parameters for the fluorine nucleus. The data were readily fit in a case (a) basis, indicating strong first order spin-orbit coupling and minimal second-order effects, as also evidenced by the small value of λ, the spin-spin parameter. Moreover, only one higher order term, η, the spin-orbit/spin-spin interaction term, was needed in the analysis, again suggesting limited perturbations in the ground state. The relative values of the a, b, and c hyperfine constants indicate that the three unpaired electrons in this radical lie in orbitals primarily located on the titanium atom and support the molecular orbital picture of TiF with a σ1δ1π1 single electron configuration. The bond length of TiF (1.8342 Å) is significantly longer than that of TiO, suggesting that there are differences in the bonding between 3d transition metal fluorides and oxides.

Yap-Hippo pathway regulates cerebral hypoxia-reoxygenation injury in neuroblastoma N2a cells via inhibiting ROCK1/F-actin/mitochondrial fission pathways.

PubMed

Geng, Chizi; Wei, Jianchao; Wu, Chengsi

2018-05-23

Yes-associated protein (Yap), a regulator of cellular apoptosis, has been demonstrated to be involved in cerebral ischemia-reperfusion (IR) injury through poorly defined mechanisms. The present study aimed to explore the role of Yap in regulating cerebral IR injury in vitro, with a focus on mitochondrial fission and ROCK1/F-actin pathways. Our data demonstrated that Yap was actually downregulated in N2a cells after cerebral hypoxia-reoxygenation (HR) injury, and that lower expression of Yap was closely associated with increased cell death. However, the reintroduction of Yap was able to suppress the HR-mediated N2a cells death via blocking the mitochondria-related apoptotic signal. At the molecular levels, Yap overexpression sustained mitochondrial potential, normalized the mitochondrial respiratory function, reduced ROS overproduction, limited HtrA2/Omi release from mitochondria into the nucleus, and suppressed pro-apoptotic proteins activation. Subsequently, functional studies have further illustrated that HR-mediated mitochondrial apoptosis was highly regulated by mitochondrial fission, whereas Yap overexpression was able to attenuate HR-mediated mitochondrial fission and, thus, promote N2a cell survival in the context of HR injury. At last, we demonstrated that Yap handled mitochondrial fission via closing ROCK1/F-actin signaling pathways. Activation of ROCK1/F-actin pathways abrogated the protective role of Yap overexpression on mitochondrial homeostasis and N2a cell survival in the setting of HR injury. Altogether, our data identified Yap as the endogenous defender to relieve HR-mediated nerve damage via antagonizing ROCK1/F-actin/mitochondrial fission pathways.

Fission fragment charge and mass distributions in 239Pu(n ,f ) in the adiabatic nuclear energy density functional theory

NASA Astrophysics Data System (ADS)

Regnier, D.; Dubray, N.; Schunck, N.; Verrière, M.

2016-05-01

Background: Accurate knowledge of fission fragment yields is an essential ingredient of numerous applications ranging from the formation of elements in the r process to fuel cycle optimization for nuclear energy. The need for a predictive theory applicable where no data are available, together with the variety of potential applications, is an incentive to develop a fully microscopic approach to fission dynamics. Purpose: In this work, we calculate the pre-neutron emission charge and mass distributions of the fission fragments formed in the neutron-induced fission of 239Pu using a microscopic method based on nuclear density functional theory (DFT). Methods: Our theoretical framework is the nuclear energy density functional (EDF) method, where large-amplitude collective motion is treated adiabatically by using the time-dependent generator coordinate method (TDGCM) under the Gaussian overlap approximation (GOA). In practice, the TDGCM is implemented in two steps. First, a series of constrained EDF calculations map the configuration and potential-energy landscape of the fissioning system for a small set of collective variables (in this work, the axial quadrupole and octupole moments of the nucleus). Then, nuclear dynamics is modeled by propagating a collective wave packet on the potential-energy surface. Fission fragment distributions are extracted from the flux of the collective wave packet through the scission line. Results: We find that the main characteristics of the fission charge and mass distributions can be well reproduced by existing energy functionals even in two-dimensional collective spaces. Theory and experiment agree typically within two mass units for the position of the asymmetric peak. As expected, calculations are sensitive to the structure of the initial state and the prescription for the collective inertia. We emphasize that results are also sensitive to the continuity of the collective landscape near scission. Conclusions: Our analysis confirms that the adiabatic approximation provides an effective scheme to compute fission fragment yields. It also suggests that, at least in the framework of nuclear DFT, three-dimensional collective spaces may be a prerequisite to reach 10% accuracy in predicting pre-neutron emission fission fragment yields.

Skyrme forces and the fusion-fission dynamics of the 132Sn+64Ni→196Pt* reaction

NASA Astrophysics Data System (ADS)

Jain, Deepika; Kumar, Raj; Sharma, Manoj K.; Gupta, Raj K.

2012-02-01

The dependence of the fusion-fission process on Skyrme forces is studied by using the dynamical cluster-decay model (DCM) and the ℓ-summed extended-Wong model in the 132Sn+64Ni→196Pt* reaction, where the nuclear proximity potential is obtained by using the semiclassical extended Thomas-Fermi (ETF) approach in the Skyrme energy density formalism (SEDF) under the frozen density approximation. The DCM gives an excellent fit to the measured fusion evaporation residue (ER) and the fission cross sections below and above barrier energies, with ER data needing “barrier lowering” at below-barrier energies for each Skyrme force (an in-built property of the DCM). The fission cross sections show a contribution of quasifission (qf) at the above-barrier two or three highest energies, depending on the Skyrme force. Calculations are illustrated for three Skyrme forces, GSkI, SSk, and SIII. Another interesting result is that there is a change of fission mass distribution from a predominantly asymmetric one to a symmetric one with a decrease in the N/Z ratio of the compound nucleus, independent of the choice of nuclear interaction potential, which gives an opportunity to address the isospin effects in the Pt* nucleus. Within the ℓ-summed extended-Wong model we find that the GSkI and SSk forces fit the total fusion cross-section data exactly, whereas the SIII force needs “barrier modification” in order to fit the data at below-barrier energies. This happens because the isospin and neutron-proton asymmetry nature of GSkI and SSk forces is different from that of the SIII force, and because the center-of-mass energy Ec.m. dependence of the barrier height for the SIII force and that of Blocki [Ann. Phys. (NY)10.1016/0003-4916(77)90249-4 105, 427 (1977)] differs strongly (by a constant amount of ˜7 MeV) from those for GSKI and SSk forces. Note that, because of the associated preformation factor with each fragment, the DCM has the advantage of treating various decay processes separately, whereas the Wong model describes only the total fusion cross section, a sum of cross sections due to all contributing processes.

Number-Theory in Nuclear-Physics in Number-Theory: Non-Primality Factorization As Fission VS. Primality As Fusion; Composites' Islands of INstability: Feshbach-Resonances?

NASA Astrophysics Data System (ADS)

Smith, A.; Siegel, Edward Carl-Ludwig

2011-03-01

Numbers: primality/indivisibility/non-factorization versus compositeness/divisibility/ factorization, often in tandem but not always, provocatively close analogy to nuclear-physics: (2 + 1)=(fusion)=3; (3+1)=(fission)=4[=2 x 2]; (4+1)=(fusion)=5; (5 +1)=(fission)=6[=2 x 3]; (6 + 1)=(fusion)=7; (7+1)=(fission)=8[= 2 x 4 = 2 x 2 x 2]; (8 + 1) =(non: fission nor fusion)= 9[=3 x 3]; then ONLY composites' Islands of fusion-INstability: 8, 9, 10; then 14, 15, 16, ... Could inter-digit Feshbach-resonances exist??? Possible applications to: quantum-information/ computing non-Shore factorization, millennium-problem Riemann-hypotheses proof as Goodkin BEC intersection with graph-theory "short-cut" method: Rayleigh(1870)-Polya(1922)-"Anderson"(1958)-localization, Goldbach-conjecture, financial auditing/accounting as quantum-statistical-physics; ...abound!!! Watkins [www.secamlocal.ex.ac.uk/people/staff/mrwatkin/] "Number-Theory in Physics" many interconnections: "pure"-maths number-theory to physics including Siegel [AMS Joint Mtg.(2002)-Abs.# 973-60-124] inversion of statistics on-average digits' Newcomb(1881)-Weyl(14-16)-Benford(38)-law to reveal both the quantum and BEQS (digits = bosons = digits:"spinEless-boZos"). 1881 1885 1901 1905 1925 < 1927, altering quantum-theory history!!!

Thermodynamics of fission products in dispersion fuel designs - first principles modeling of defect behavior in bulk and at interfaces

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Xiang-yand; Uberuaga, Blas P; Nerikar, Pankaj

2009-01-01

Density functional theory (DFT) calculations of fission product (Xe, Sr, and Cs) incorporation and segregation in alkaline earth metal oxides, HfO{sub 2} and UO{sub 2} oxides, and the MgO/(U, Hf, Ce)O{sub 2} interfaces have been carried out. In the case of UO{sub 2}, the calculations were performed using spin polarization and with a Hubbard U term characterizing the on-sit Coulomb repulsion between the localized 5f electrons. The fission product solution energies in bulk UO{sub 2{+-}x} have been calculated as a function of non-stoichiometry x, and were compared to that in MgO. These calculations demonstrate that the fission product incorporation energiesmore » in MgO are higher than in HfO{sub 2}. However, this trend is reversed or reduced for alkaline earth oxides with larger cation sizes. The solution energies of fission products in MgO are substantially higher than in UO{sub 2{+-}x}, except for the case of Sr in the hypostoichiometric case. Due to size effects, the thermodynamic driving force of segregation for Xe and Cs from bulk MgO to the MgO/fluorite interface is strong. However, this driving force is relatively weak for Sr.« less

Effects of the Electronic Spin-Orbit Interaction on the Anomalous Asymmetric Scattering of the Spin-Polarized He+ Beam with Paramagnetic Target Materials II. Partial Wave Representation

NASA Astrophysics Data System (ADS)

Sakai, Osamu; Suzuki, Taku T.

2018-05-01

The scattering of an electron-spin-polarized 4He+ beam on paramagnetic materials has an anomalously large asymmetric scattering component (ASC) around 10%, which is 104 times that expected from the spin-orbit coupling for the potential of the target nucleus. The scattering angle (θ) dependence of the ASC has been measured. It changes sign near 90° for some materials (for example, Au and Pt), while it does not change sign for other materials (for example, Pb and Bi). It has been noted that the spin-orbit interaction of electrons on the target in the electron-transfer intermediate state causes the ASC of He nucleus motion, and it has also been predicted that the sign change in the θ dependence occurs when the d electron transfer is dominant. This seems to correspond to the cases of Au and Pt, but not to the cases of Pb and Bi. The previous approach is refined on the basis of the partial wave representation, which can give a more correct estimation of the ASC. It is shown that the sign change appears in the weak-resonance domain in the case of d electron excitation, whereas the sign change disappears in the strong-resonance domain. Our calculated results qualitatively agree with the material dependence of the ASC observed experimentally.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kadmensky, S. G., E-mail: kadmensky@phys.vsu.ru; Kostryukov, P. V.

It is shown that a quantum system whose Hamiltonian is independent of time is T -invariant if this Hamiltonian contains only those terms that do not change sign upon time reversal. It is also shown that the coincidence of the amplitudes for multistep direct and statistical nuclear reactions with the timereversed amplitudes for the reactions being studied is a condition that ensures the T -invariance of the amplitudes in question, the transition from the original amplitudes to their time-reversed counterparts being accomplished, first, upon introducing the inverse-reactionmatrices T instead of the original-reaction matrix T and, second, upon replacing the wavemore » functions for the initial, final, and intermediate states of the system by the respective time-reversed functions. It is found that the T -even (T -odd) asymmetries in cross sections for nuclear reactions stem from the interference between the amplitudes characterizing these reactions and having identical (opposite) T -parities. It is shown that the T -invariance condition for the above T -even (T -odd) asymmetries is related to the conservation of (change in) the sign of these asymmetries upon going over from original to inverse nuclear reactions. Mechanisms underlying the appearance of possible T -even and T-odd asymmetries in the cross sections for the cold-polarizedneutron- induced binary and ternary fission of oriented target nuclei are analyzed for the case of employing T -invariant Hamiltonians for the systems under study. It is also shown that the asymmetries in question satisfy the T -invariance condition if the reactions being considered have a sequential multistep statistical character. It is concluded that T -invariance is violated in the limiting case where, in ternary nuclear fission, the emission of a light third particle froma fissile compound nucleus formed upon incident-neutron capture by a target nucleus and its separation to two fission fragments are simultaneous events.« less

International Halley Watch: Discipline specialists for near-nucleus studies

NASA Technical Reports Server (NTRS)

Larson, S.; Sekanina, Z.; Rahe, J.

1986-01-01

The purpose of the Near-Nucleus Studies Net is to study the processes taking place in the near-nucleus environment as they relate to the nature of nucleus. This is accomplisghed by measuring the spatial and temporal distribution of dust, gases and ions in the coma on high resolution images taken from many observatories around the world. By modeling the motions of discrete dust features in Comet Halley, it is often possible to determine the locations of the emission sources on the surface and learn about the nucleus structure. In addition to the general goals shared by all IHW nets, the scientific goals of the net has been to determine (1)the gross surface structure of the nucleus, (2)the nucleus spin vector, (3)the distribution and evolution of jet sources and (4)the interrelationships between the gas, dust and ion components of the coma. An additional Comet Giacobini-Zinner watch was carried out by the NNSN in support of the NASA International Cometary Explorer flyby.

Single-particle excitations in the level structure of 64Cu

NASA Astrophysics Data System (ADS)

Samanta, S.; Das, S.; Bhattacharjee, R.; Chatterjee, S.; Raut, R.; Ghugre, S. S.; Sinha, A. K.; Garg, U.; Neelam, Kumar, N.; Jones, P.; Laskar, Md. Sazedur R.; Babra, F. S.; Biswas, S.; Saha, S.; Singh, P.; Palit, R.

2018-01-01

Excited states of the 64Cu(Z =29 ,N =35 ) nucleus have been probed using heavy-ion-induced fusion evaporation reaction and an array of Compton-suppressed Clovers as detection system for the emitted γ rays. More than 50 new transitions have been identified and the level scheme of the nucleus has been established up to an excitation energy Ex˜6 MeV and spin ˜10 ℏ . The experimental results have been compared with those from large-basis shell-model calculations that facilitated an understanding of the single-particle configurations underlying the level structure of the nucleus.

Nuclear shape evolution based on microscopic level densities

DOE PAGES

Ward, D. E.; Carlsson, B. G.; Døssing, T.; ...

2017-02-27

Here, by combining microscopically calculated level densities with the Metropolis walk method, we develop a consistent framework for treating the energy and angular-momentum dependence of the nuclear shape evolution in the fission process. For each nucleus under consideration, the level density is calculated microscopically for each of more than five million shapes with a recently developed combinatorial method. The method employs the same single-particle levels as those used for the extraction of the pairing and shell contributions to the macroscopic-microscopic deformation-energy surface. Containing no new parameters, the treatment is suitable for elucidating the energy dependence of the dynamics of warmmore » nuclei on pairing and shell effects. It is illustrated for the fission fragment mass distribution for several uranium and plutonium isotopes of particular interest.« less

Spin excitations in the deformed nuclei 154Sm, 158Gd and 168Er

NASA Astrophysics Data System (ADS)

Frekers, D.; Wörtche, H. J.; Richter, A.; Abegg, R.; Azuma, R. E.; Celler, A.; Chan, C.; Drake, T. E.; Helmer, R.; Jackson, K. P.; King, J. D.; Miller, C. A.; Schubank, R.; Vetterli, M. C.; Yen, S.

1990-07-01

An intermediate energy proton scattering experiment has been performed to probe spin excitation in the deformed rare earth nuclei 154Sm, 158Gd and 168Er for energies up to 12 MeV. A concentration of spin M1 strength is observed between 6 and 10MeV with a total strength of about 11 μN2 independent of the nucleus. The strength function shows two distinct structures separated by about 2.5 MeV and each having a width of about 2 MeV.

Electric dipole moment of diatomic molecules by configuration interaction. V - Two states of /2/Sigma/+/ symmetry in CN.

NASA Technical Reports Server (NTRS)

Green, S.

1972-01-01

Previous accurate dipole moment calculation techniques are modified to be applicable to higher excited states of symmetry. The self-consistent fields and configuration interactions are calculated for the X(2)Sigma(+) and B(2)Sigma(+) states of CN. Spin hyperfine constants and spin density at the nucleus are considered in the context of one-electron operator properties. The values of the self-consistent field and configuration interaction for the spin density are compared with experimental values for several diatomic molecules.

Fusion-fission and quasifission of superheavy systems with Z =110 -116 formed in 48Ca-induced reactions

NASA Astrophysics Data System (ADS)

Kozulin, E. M.; Knyazheva, G. N.; Itkis, I. M.; Itkis, M. G.; Bogachev, A. A.; Chernysheva, E. V.; Krupa, L.; Hanappe, F.; Dorvaux, O.; Stuttgé, L.; Trzaska, W. H.; Schmitt, C.; Chubarian, G.

2014-11-01

Background: In heavy-ion-induced reactions the mechanism leading to the formation of the compound nucleus and the role of quasifission is still not clear. Purpose: Investigation of the quasifission process of superheavy composite systems with Z =110 -116 and comparison with properties of fusion-fission and quasifission of lighter composite systems. Method: Mass and energy distributions of fissionlike fragments formed in the reactions 48Ca+232Th, 238U , 244Pu , and 248Cm at energies near the Coulomb barrier have been measured using the double-arm time-of-flight spectrometer CORSET at the U-400 cyclotron of the FLNR JINR. Results: The most probable fragment masses as well as total kinetic energies and their dispersions in dependence on the interaction energies and ion-target combinations have been studied for asymmetric and symmetric fragments formed in the reactions. The capture cross sections were obtained for the reactions 48Ca+244Pu and 248Cm . The lower limits for fission barriers of 283 -286Cn , 289 -292Fl , and 293 -296Lv compound nuclei were estimated. Conclusions: Analysis of the properties of symmetric fragments has shown that a significant part of these fragments may be attributed to fusion-fission process for the reactions 48Ca +238U , 244Pu , and 248Cm .

Fast passage dynamic nuclear polarization on rotating solids.

PubMed

Mentink-Vigier, Frederic; Akbey, Umit; Hovav, Yonatan; Vega, Shimon; Oschkinat, Hartmut; Feintuch, Akiva

2012-11-01

Magic Angle Spinning (MAS) Dynamic Nuclear Polarization (DNP) has proven to be a very powerful way to improve the signal to noise ratio of NMR experiments on solids. The experiments have in general been interpreted considering the Solid-Effect (SE) and Cross-Effect (CE) DNP mechanisms while ignoring the influence of sample spinning. In this paper, we show experimental data of MAS-DNP enhancements of (1)H and (13)C in proline and SH3 protein in glass forming water/glycerol solvent containing TOTAPOL. We also introduce a theoretical model that aims at explaining how the nuclear polarization is built in MAS-DNP experiments. By using Liouville space based simulations to include relaxation on two simple spin models, {electron-nucleus} and {electron-electron-nucleus}, we explain how the basic MAS-SE-DNP and MAS-CE-DNP processes work. The importance of fast energy passages and short level anti-crossing is emphasized and the differences between static DNP and MAS-DNP is explained. During a single rotor cycle the enhancement in the {electron-electron-nucleus} system arises from MAS-CE-DNP involving at least three kinds of two-level fast passages: an electron-electron dipolar anti-crossing, a single quantum electron MW encounter and an anti-crossing at the CE condition inducing nuclear polarization in- or decrements. Numerical, powder-averaged, simulations were performed in order to check the influence of the experimental parameters on the enhancement efficiencies. In particular we show that the spinning frequency dependence of the theoretical MAS-CE-DNP enhancement compares favorably with the experimental (1)H and (13)C MAS-DNP enhancements of proline and SH3. Copyright © 2012 Elsevier Inc. All rights reserved.

Fusion of deformed nuclei in the reactions of 76Ge+150Nd and 28Si+198Pt at the Coulomb barrier region

NASA Astrophysics Data System (ADS)

Nishio, K.; Ikezoe, H.; Mitsuoka, S.; Lu, J.

2000-07-01

Evaporation residue cross sections for 28Si+198Pt and 76Ge+150Nd, both of which form a compound nucleus 226U, were measured in the vicinity of the Coulomb barrier. The measurement gives direct evidence that the system really fuses together to form a fully equilibrated compound nucleus. For the 28Si+198Pt reaction, we have measured the fission fragments to determine the fusion cross section by taking advantage of the highly fissile character of 226U. The evaporation residue cross section and the fusion cross section for 28Si+198Pt allowed us to investigate the deexcitation process (exit channel) of the compound nucleus 226U, and the parameters entering in a statistical model calculation could be determined. By estimating the deexcitation of the compound nucleus 226U with the statistical model, the effect of the deformed nucleus 150Nd on the fusion reaction 76Ge+150Nd was extracted. The experimental data indicated that there is more than 13 MeV extra-extra-push energy for the system to fuse together when the projectile 76Ge collides at the tip of the deformed 150Nd nucleus. On the contrary, for the side collision which is more compact in configuration than the tip collision, no fusion hindrance is suggested.

Rolf Landauer and Charles H. Bennett Award Talk: Experimental development of spin qubits in silicon

NASA Astrophysics Data System (ADS)

Morello, Andrea

The modern information era is built on silicon nanoelectronic devices. The future quantum information era might be built on silicon too, if we succeed in controlling the interactions between individual spins hosted in silicon nanostructures. Spins in silicon constitute excellent solid-state qubits, because of the weak spin-orbit coupling and the possibility to remove nuclear spins from the environment through 28Si isotopic enrichment. Substitutional 31P atoms in silicon behave approximately like hydrogen in vacuum, providing two spin 1/2 qubits - the donor-bound electron and the 31P nucleus - that can be coherently controlled, read out in single-shot, and are naturally coupled through the hyperfine interaction. In isotopically-enriched 28Si, these single-atom qubits have demonstrated outstanding coherence times, up to 35 seconds for the nuclear spin, and 1-qubit gate fidelities well above 99.9% for both the electron and the nucleus. The hyperfine coupling provides a built-in interaction to entangle the two qubits within one atom. The combined initialization, control and readout fidelities result in a violation of Bell's inequality with S = 2 . 70 , a record value for solid-state qubits. Despite being identical atomic systems, 31P atoms can be addressed individually by locally modifying the hyperfine interaction through electrostatic gating. Multi-qubit logic gates can be mediated either by the exchange interaction or by electric dipole coupling. Scaling up beyond a single atom presents formidable challenges, but provides a pathway to building quantum processors that are compatible with standard semiconductor fabrication, and retain a nanometric footprint, important for truly large-scale quantum computers. Work supported by US Army Research Office (W911NF-13-1-0024) and Australian Research Council (CE110001027).

Protoearth mass shedding and the origin of the moon

NASA Technical Reports Server (NTRS)

Boss, A. P.

1986-01-01

Darwin's (1980) theory of lunar formation from the earth by means of a rotationally driven dynamic fission instability is presently considered in view of viscous shear's maintenance of solid body rotation throughout the protoearth's accretion phase. Assuming the appropriateness of a polytropic account of the protoearth, it is unlikely that dynamic fission could have occurred; instantaneous spin-up following a giant impact would instead have led to mass shedding. The dynamical phenomenon of mass shedding is here explored on the basis of numerical models for a self-gravitating, axisymmetric, polytropic and dissipative protoearth. It is concluded that mass shedding from the protoearth mantle after a giant impact and explosion could have contributed substantial matter to a lunar disk.

Synthesis reactions and radioactive properties of transactinoid elements

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.

1994-10-01

It is well known that the heaviest elements of the periodic table have been synthesized in the cold fusion of magic nuclei of Pb with Z less than 26 ions. Because of dynamic limitations for fusion under strong Coulomb interaction of nuclei, the cross-sections of cold fusion reactions diminish exponentially with growing compound nucleus atomic number. For element Z = 110 produced in the reaction Pb-208(Ni-62,n)(sub 271)110, the expected cross-section is 10(exp -36) sq cm. In still more asymmetric reactions, when isotopes of actinoid elements irradiated with relatively light ions (Z less than or equal 12) are used as the target material, the compound nuclei possess an excitation energy of approx. 50 MeV. At this energy the nuclear shell effects are strongly suppressed and, as a result, in the case of hot compound nuclei of transactinoid elements the fission barrier is practically absent. The transition of these nuclei into the ground state depends strongly on the dynamic properties of the system with respect to the fission degree of freedom. Experimental studies were going on in two directions: (1) determination of the fission time by measuring the prefission neutrons (of Cf-Fm nuclei) in a wide interval of excitation energies; (2) direct synthesis of known nuclides with Z = 102-105 in reactions with ions of Ne-22, Mg-26, Al-27 and P-31 when final nuclei are produced in the ground state after the evaporation of five or six neutrons from the excited compound nuclei (E(sub x) = 50-60 MeV). The dependence of the reaction cross-section (HI, 5-6n) on the atomic number of the compound nucleus in different target-ion combinations points to the possibility of synthesizing new elements in hot fusion reactions. The advantage of these reactions arises from the use of neutron-rich nuclei like Cm-248 and Cf-249 which allows us to synthesize nuclei close to the deformed shell N = 162, for which a considerable growth of stability against spontaneous fission is predicted. Experimental set-ups and methods of detecting rare events of formation and decay of transactinide nuclei are described.

Spin-dependent evolution of collectivity in 112Te

NASA Astrophysics Data System (ADS)

Doncel, M.; Bäck, T.; Qi, C.; Cullen, D. M.; Hodge, D.; Cederwall, B.; Taylor, M. J.; Procter, M.; Giles, M.; Auranen, K.; Grahn, T.; Greenlees, P. T.; Jakobsson, U.; Julin, R.; Juutinen, S.; HerzáÅ, A.; Konki, J.; Pakarinen, J.; Partanen, J.; Peura, P.; Rahkila, P.; Ruotsalainen, P.; Sandzelius, M.; Sarén, J.; Scholey, C.; Sorri, J.; Stolze, S.; Uusitalo, J.

2017-11-01

The evolution of collectivity with spin along the yrast line in the neutron-deficient nucleus 112Te has been studied by measuring the reduced transition probability of excited states in the yrast band. In particular, the lifetimes of the 4+ and 6+ excited states have been determined by using the recoil distance Doppler-shift method. The results are discussed using both large-scale shell-model and total Routhian surface calculations.

Indirect detection of 10B (I = 3) overtone NMR at very fast magic angle spinning

NASA Astrophysics Data System (ADS)

Duong, Nghia Tuan; Kuprov, Ilya; Nishiyama, Yusuke

2018-06-01

The application of overtone nuclear magnetic resonance (OT NMR) to symmetric spin transitions of integer quadrupolar nuclei is of considerable interest since this transition is immune to the first-order quadrupolar interaction, thus resulting in narrow NMR lines. Owing to its roles in nature and its high natural abundance, 14N (I = 1) OT NMR has been explored, in which the indirect and/or direct acquisitions of 14N OT were experimentally demonstrated. However, other than 14N nucleus, no OT NMR observation of other integer quadrupolar nuclei has been reported in the literature. In this work, we extend the application of OT NMR to another integer quadrupolar nucleus, namely 10B (I = 3). However, this is not straightforward owing to the unfavorable characteristics of 10B isotope. Here, for the first time, we present the selective acquisition of 10B central (-1 ↔ +1) OT NMR via detection of 1H nuclei on perborate monohydrate sample. Numerical calculations are in a good agreement with the experimental results. Both show that the optimal sensitivity is achieved when the carrier frequency is applied at the second OT spinning sideband, i.e. an offset of twice of the spinning frequency from the center band.

Toroidal high-spin isomers in the nucleus 304120

NASA Astrophysics Data System (ADS)

Staszczak, A.; Wong, Cheuk-Yin; Kosior, A.

2017-05-01

Background: Strongly deformed oblate superheavy nuclei form an intriguing region where the toroidal nuclear structures may bifurcate from the oblate spheroidal shape. The bifurcation may be facilitated when the nucleus is endowed with a large angular moment about the symmetry axis with I =Iz . The toroidal high-K isomeric states at their local energy minima can be theoretically predicted using the cranked self-consistent Skyrme-Hartree-Fock method. Purpose: We use the cranked Skyrme-Hartree-Fock method to predict the properties of the toroidal high-spin isomers in the superheavy nucleus 120304184. Method: Our method consists of three steps: First, we use the deformation-constrained Skyrme-Hartree-Fock-Bogoliubov approach to search for the nuclear density distributions with toroidal shapes. Next, using these toroidal distributions as starting configurations, we apply an additional cranking constraint of a large angular momentum I =Iz about the symmetry z axis and search for the energy minima of the system as a function of the deformation. In the last step, if a local energy minimum with I =Iz is found, we perform at this point the cranked symmetry- and deformation-unconstrained Skyrme-Hartree-Fock calculations to locate a stable toroidal high-spin isomeric state in free convergence. Results: We have theoretically located two toroidal high-spin isomeric states of 120304184 with an angular momentum I =Iz=81 ℏ (proton 2p-2h, neutron 4p-4h excitation) and I =Iz=208 ℏ (proton 5p-5h, neutron 8p-8h) at the quadrupole moment deformations Q20=-297.7 b and Q20=-300.8 b with energies 79.2 and 101.6 MeV above the spherical ground state, respectively. The nuclear density distributions of the toroidal high-spin isomers 120304184(Iz=81 ℏ and 208 ℏ ) have the maximum density close to the nuclear matter density, 0.16 fm-3, and a torus major to minor radius aspect ratio R /d =3.25 . Conclusions: We demonstrate that aligned angular momenta of Iz=81 ℏ and 208 ℏ arising from multiparticle-multihole excitations in the toroidal system of 120304184 can lead to high-spin isomeric states, even though the toroidal shape of 120304184 without spin is unstable. Toroidal energy minima without spin may be possible for superheavy nuclei with higher atomic numbers, Z ≳122 , as reported previously [7 A. Staszczak and C. Y. Wong, Acta Phys. Pol. B 40, 753 (2008)].

Toroidal high-spin isomers in the nucleus 120 304

DOE PAGES

Staszczak, A.; Wong, Cheuk-Yin; Kosior, A.

2017-05-22

Strongly deformed oblate superheavy nuclei form an intriguing region where the toroidal nuclear structures may bifurcate from the oblate spheroidal shape. The bifurcation may be facilitated when the nucleus is endowed with a large angular moment about the symmetry axis withmore » $$I=I_{z}$$. The toroidal high-$K$ isomeric states at their local energy minima can be theoretically predicted using the cranked self-consistent Skyrme-Hartree-Fock method. We use the cranked Skyrme-Hartree-Fock method to predict the properties of the toroidal high-spin isomers in the superheavy nucleus $$^{304}{120}_{184}$$. This method consists of three steps: first, we use the deformation-constrained Skyrme-Hartree-Fock-Bogoliubov approach to search for the nuclear density distributions with toroidal shapes. Next, using these toroidal distributions as starting configurations we apply an additional cranking constraint of a large angular momentum $$I=I_{z}$$ about the symmetry $z$-axis and search for the energy minima of the system as a function of the deformation. In the last step, if a local energy minimum with $$I=I_{z}$$ is found, we perform at this point the cranked symmetry- and deformation-unconstrained Skyrme-Hartree-Fock calculations to locate a stable toroidal high-spin isomeric state in free convergence. Furthemore, we have theoretically located two toroidal high-spin isomeric states of $$^{304}{120}_{184}$$ with an angular momentum $I$=$$I_z$$=81$$\\hbar$$ (proton 2p-2h, neutron 4p-4h excitation) and $I$=$$I_z$$=208$$\\hbar$$ (proton 5p-5h, neutron 8p-8h) at the quadrupole moment deformations $$Q_{20}=-297.7$$~b and $$Q_{20}=-300.8$$~b with energies 79.2 MeV and 101.6 MeV above the spherical ground state, respectively. The nuclear density distributions of the toroidal high-spin isomers $$^{304}{120}_{184}(I_z$$=81$$\\hbar$$ and 208$$\\hbar$$) have the maximum density close to the nuclear matter density, 0.16 fm$$^{-3}$$, and a torus major to minor radius aspect ratio $R/d=3.25$. Here, we demonstrate that aligned angular momenta of $$I_z$$=81$$\\hbar$$ and 208$$\\hbar$$ arising from multi-particle-multi-hole excitations in the toroidal system of $$^{304}{120}_{184}$$ can lead to high-spin isomeric states, even though the toroidal shape of $$^{304}120_{184}$$ without spin is unstable. Toroidal energy minima without spin may be possible for superheavy nuclei with higher atomic numbers, $$Z\\gtrsim$$122, as reported previously [A. Staszczak and C. Y. Wong,Acta Phys. Pol. B 40 , 753 (2008)].« less

Can reliable values of Young's modulus be deduced from Fisher's (1971) spinning lens measurements?

PubMed

Burd, H J; Wilde, G S; Judge, S J

2006-04-01

The current textbook view of the causes of presbyopia rests very largely on a series of experiments reported by R.F. Fisher some three decades ago, and in particular on the values of lens Young's modulus inferred from the deformation caused by spinning excised lenses about their optical axis (Fisher 1971) We studied the extent to which inferred values of Young's modulus are influenced by assumptions inherent in the mathematical procedures used by Fisher to interpret the test and we investigated several alternative interpretation methods. The results suggest that modelling assumptions inherent in Fisher's original method may have led to systematic errors in the determination of the Young's modulus of the cortex and nucleus. Fisher's conclusion that the cortex is stiffer than the nucleus, particularly in middle age, may be an artefact associated with these systematic errors. Moreover, none of the models we explored are able to account for Fisher's claim that the removal of the capsule has only a modest effect on the deformations induced in the spinning lens.

Dynamical Cluster-decay Model (DCM) applied to 9Li+208Pb reaction

NASA Astrophysics Data System (ADS)

Kaur, Arshdeep; Hemdeep; Kaushal, Pooja; Behera, Bivash R.; Gupta, Raj K.

2017-10-01

The decay mechanism of 217At* formed in 9Li+208Pb reaction is studied within the dynamical cluster-decay model (DCM) at various center-of-mass energies. The aim is to see the behavior of a light neutron-rich radioactive beam on a doubly-magic target nucleus for the (total) fusion cross section σfus and the individual decay channel cross sections. Experimentally, only the isotopic yield of heavy mass residues * 211- 214At [equivalently, the light-particles (LPs) evaporation residue cross sections σxn for x = 3- 6 neutrons emission] are measured, with the fusion-fission (ff) component σff taken zero. For a fixed neck-length parameter ΔR, the only parameter in the DCM, we are able to fit σfus =∑x=16σxn almost exactly for 9Li on 208Pb at all E c . m .'s. However, the observed individual decay channels (3n-6n) are very poorly fitted, with unobserved channels (1n, 2n) and σff strongly over-estimated. Different ΔR values, meaning thereby different reaction time scales, are required to fit individually both the observed and unobserved evaporation residue channels (1n-6n) and σff, but then the compound nucleus (CN) contribution σCN is very small (< 1%), and the non-compound nucleus (nCN) decay cross section σnCN contributes the most towards total σfus (=σCN +σnCN). Thus, the 9Li induced reaction on doubly-magic 208Pb is more of a quasi-fission-like nCN decay, which is further analyzed in terms of the statistical CN formation probability PCN and CN survival probability Psurv. For the reaction under study, PCN < < 1 and Psurv → 1, in particular at above barrier energies.

Dynamic nuclear polarization assisted spin diffusion for the solid effect case.

PubMed

Hovav, Yonatan; Feintuch, Akiva; Vega, Shimon

2011-02-21

The dynamic nuclear polarization (DNP) process in solids depends on the magnitudes of hyperfine interactions between unpaired electrons and their neighboring (core) nuclei, and on the dipole-dipole interactions between all nuclei in the sample. The polarization enhancement of the bulk nuclei has been typically described in terms of a hyperfine-assisted polarization of a core nucleus by microwave irradiation followed by a dipolar-assisted spin diffusion process in the core-bulk nuclear system. This work presents a theoretical approach for the study of this combined process using a density matrix formalism. In particular, solid effect DNP on a single electron coupled to a nuclear spin system is considered, taking into account the interactions between the spins as well as the main relaxation mechanisms introduced via the electron, nuclear, and cross-relaxation rates. The basic principles of the DNP-assisted spin diffusion mechanism, polarizing the bulk nuclei, are presented, and it is shown that the polarization of the core nuclei and the spin diffusion process should not be treated separately. To emphasize this observation the coherent mechanism driving the pure spin diffusion process is also discussed. In order to demonstrate the effects of the interactions and relaxation mechanisms on the enhancement of the nuclear polarization, model systems of up to ten spins are considered and polarization buildup curves are simulated. A linear chain of spins consisting of a single electron coupled to a core nucleus, which in turn is dipolar coupled to a chain of bulk nuclei, is considered. The interaction and relaxation parameters of this model system were chosen in a way to enable a critical analysis of the polarization enhancement of all nuclei, and are not far from the values of (13)C nuclei in frozen (glassy) organic solutions containing radicals, typically used in DNP at high fields. Results from the simulations are shown, demonstrating the complex dependences of the DNP-assisted spin diffusion process on variations of the relevant parameters. In particular, the effect of the spin lattice relaxation times on the polarization buildup times and the resulting end polarization are discussed, and the quenching of the polarizations by the hyperfine interaction is demonstrated.

Long-lived K isomer and enhanced γ vibration in the neutron-rich nucleus 172Dy: Collectivity beyond double midshell

NASA Astrophysics Data System (ADS)

Watanabe, H.; Zhang, G. X.; Yoshida, K.; Walker, P. M.; Liu, J. J.; Wu, J.; Regan, P. H.; Söderström, P.-A.; Kanaoka, H.; Korkulu, Z.; Lee, P. S.; Nishimura, S.; Yagi, A.; Ahn, D. S.; Alharbi, T.; Baba, H.; Browne, F.; Bruce, A. M.; Carroll, R. J.; Chae, K. Y.; Dombradi, Zs.; Doornenbal, P.; Estrade, A.; Fukuda, N.; Griffin, C.; Ideguchi, E.; Inabe, N.; Isobe, T.; Kanaya, S.; Kojouharov, I.; Kondev, F. G.; Kubo, T.; Kubono, S.; Kurz, N.; Kuti, I.; Lalkovski, S.; Lane, G. J.; Lee, C. S.; Lee, E. J.; Lorusso, G.; Lotay, G.; Moon, C.-B.; Nishizuka, I.; Nita, C. R.; Odahara, A.; Patel, Z.; Phong, V. H.; Podolyák, Zs.; Roberts, O. J.; Sakurai, H.; Schaffner, H.; Shand, C. M.; Shimizu, Y.; Sumikama, T.; Suzuki, H.; Takeda, H.; Terashima, S.; Vajta, Zs.; Valiente-Dóbon, J. J.; Xu, Z. Y.

2016-09-01

The level structure of 172Dy has been investigated for the first time by means of decay spectroscopy following in-flight fission of a 238U beam. A long-lived isomeric state with T1/2 = 0.71 (5) s and Kπ =8- has been identified at 1278 keV, which decays to the ground-state and γ-vibrational bands through hindered electromagnetic transitions, as well as to the daughter nucleus 172Ho via allowed β decays. The robust nature of the Kπ =8- isomer and the ground-state rotational band reveals an axially-symmetric structure for this nucleus. Meanwhile, the γ-vibrational levels have been identified at unusually low excitation energy compared to the neighboring well-deformed nuclei, indicating the significance of the microscopic effect on the non-axial collectivity in this doubly mid-shell region. The underlying mechanism of enhanced γ vibration is discussed in comparison with the deformed Quasiparticle Random-Phase Approximation based on a Skyrme energy-density functional.

Basic distinctions between cold- and hot-fusion reactions in the synthesis of superheavy elements

NASA Astrophysics Data System (ADS)

Nasirov, A. K.; Muminov, A. I.; Giardina, G.; Mandaglio, G.

2014-07-01

Superheavy elements (SHE) of charge number in the range of Z = 106-112 were synthesized in so-called cold-fusion reactions. The smallness of the excitation energy of compound nuclei is the main advantage of cold-fusion reactions. However, the synthesis of SHEs of charge number in the region of Z ≥ 112 is strongly complicated in cold-fusion reactions by a sharp decrease in the cross section of a compound nucleus formation in the entrance channel because of superiority of quasifission in the competition with complete fusion. Two favorable circumstances contributed to the success of the experiments aimed at the synthesis of the Z = 113-118 elements and performed at the Laboratory of Nuclear Reactions at the Joint Institute for Nuclear Research: large cross sections for the production of a compound nucleus, which are characteristic of hot-fusion reactions, and an increase in the fission barrier for nuclei toward the stability island. The factor that complicates the formation of a compound nucleus in cold-fusion reactions is discussed.

The Demonstration of the Feasibility of the Tuning and Stimulation of Nuclear Radiation.

DTIC Science & Technology

1988-10-31

line, or the center of a resonance pattern, is called the isomer shift. It is due to the electrostatic interaction of the nucleus with the electron ...magnetic moment due to the presence of unpaired electrons , the material is either paramagnetic or ferromagnetic. In paramagnetic materials these moments...capture and fission.4,5,8 A very fertile interdisciplinary area of nuclear quantum electronics 7 appeared to be developing, encouraged by the

Stardust-NExT, Deep Impact, and the Accelerating Spin of 9P/Tempel 1

NASA Technical Reports Server (NTRS)

Belton, Michael J. S.; Meech, Karen J.; Chesley, Steven; Pittichova, Jana; Carcich, Brian; Drahus, Michal; Harris, Alan; Gillam, Stephen; Veverka, Joseph; Mastrodemos, Nicholas;

Stardust-NExT, Deep Impact, and the Accelerating Spin of 9P/Tempel One

NASA Technical Reports Server (NTRS)

Belton, Michael J. S.; Meech, Karen J.; Chesley, Steven; Pittichova, Jana; Carcich, Brian; Drahus, Michal; Harris, Alan; Gillam, Stephen; Veverka, Joseph; A'Hearn, Michael F.;

A Monte Carlo Simulation of Prompt Gamma Emission from Fission Fragments

NASA Astrophysics Data System (ADS)

Regnier, D.; Litaize, O.; Serot, O.

2013-03-01

The prompt fission gamma spectra and multiplicities are investigated through the Monte Carlo code FIFRELIN which is developed at the Cadarache CEA research center. Knowing the fully accelerated fragment properties, their de-excitation is simulated through a cascade of neutron, gamma and/or electron emissions. This paper presents the recent developments in the FIFRELIN code and the results obtained on the spontaneous fission of 252Cf. Concerning the decay cascades simulation, a fully Hauser-Feshbach model is compared with a previous one using a Weisskopf spectrum for neutron emission. A particular attention is paid to the treatment of the neutron/gamma competition. Calculations lead using different level density and gamma strength function models show significant discrepancies of the slope of the gamma spectra at high energy. The underestimation of the prompt gamma spectra obtained regardless our de-excitation cascade modeling choice is discussed. This discrepancy is probably linked to an underestimation of the post-neutron fragments spin in our calculation.

Magnetic Moment of Proton Drip-Line Nucleus (9)C

NASA Technical Reports Server (NTRS)

Matsuta, K.; Fukuda, M.; Tanigaki, M.; Minamisono, T.; Nojiri, Y.; Mihara, M.; Onishi, T.; Yamaguchi, T.; Harada, A.; Sasaki, M.

1994-01-01

The magnetic moment of the proton drip-line nucleus C-9(I(sup (pi)) = 3/2, T(sub 1/2) = 126 ms) has been measured for the first time, using the beta-NMR detection technique with polarized radioactive beams. The measure value for the magnetic moment is 1mu(C-9)! = 1.3914 +/- 0.0005 (mu)N. The deduced spin expectation value of 1.44 is unusually larger than any other ones of even-odd nuclei.

From the Old to the New World of Nuclear Physics

NASA Astrophysics Data System (ADS)

Stuewer, Roger H.

Physicists passed from the Old to the New World of Nuclear Physics in the two decades between the first and second world wars. The transition occurred against the background of the Great War, the postwar hyperinflation in Germany and Austria, and the greatest intellection migrations in history after the Nazi Civil Service law of 1933, the Anschlussof Austria in March 1938, and the Fascist anti-Semitic laws that fall. It involved Rutherford's discovery of artificial disintegration, Pettersson and Kirsch's challenge of it, and the concomitant rise and fall of Rutherford's satellite model of the nucleus; Gamow's quantum-mechanical theory of alpha decay and his liquid-drop model of the nucleus; the discoveries of deuterium and the deuteron, neutron, and positron, and the inventions of the Cockcroft-Walton accelerator and the cyclotron; the influence of the seventh Solvay Conference; Joliot and Curie's discovery of artificial radioactivity; Pauli's neutrino hypothesis, Fermi's theory of beta decay, and his discovery of the efficacy of slow neutrons in producing nuclear reactions; Bohr's theory of the compound nucleus and Breit and Wigner's theory of neutron-nucleus resonances; and the discovery of nuclear fission, Meitner and Frisch's interpretation of it, and Bohr and Fermi revelation of both in America.

Cement As a Waste Form for Nuclear Fission Products: The Case of 90Sr and Its Daughters [Cement As a Container for Nuclear Fission Products: The Case of 90Sr and Its Daughters

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dezerald, Lucile; Kohanoff, Jorge J.; Correa, Alfredo A.

One of the main challenges faced by the nuclear industry is the long-term confinement of nuclear waste. Because it is inexpensive and easy to manufacture, cement is the material of choice to store large volumes of radioactive materials, in particular the low-level medium-lived fission products. It is therefore of utmost importance to assess the chemical and structural stability of cement containing radioactive species. Here, we use ab initio calculations based on density functional theory (DFT) to study the effects of 90Sr insertion and decay in C–S–H (calcium-silicate-hydrate) in order to test the ability of cement to trap and hold thismore » radioactive fission product and to investigate the consequences of its β-decay on the cement paste structure. We show that 90Sr is stable when it substitutes the Ca 2+ ions in C–S–H, and so is its daughter nucleus 90Y after β-decay. Interestingly, 90Zr, daughter of 90Y and final product in the decay sequence, is found to be unstable compared to the bulk phase of the element at zero K but stable when compared to the solvated ion in water. Furthermore, cement appears as a suitable waste form for 90Sr storage.« less

Spontaneous fission of the end product in α-decay chain of recoiled superheavy nucleus: A theoretical study

NASA Astrophysics Data System (ADS)

Kaur, Amandeep; Sawhney, Gudveen; Sharma, Manoj K.; Gupta, Raj K.

The temperature-dependent preformed cluster model [PCM(T)] is employed to extend our recent work [Niyti, G. Sawhney, M. K. Sharma and R. K. Gupta, Phys. Rev. C 91 (2015) 054606] on α-decay chains of various isotopes of Z = 113-118 superheavy nuclei (SHN), to spontaneous fissioning nuclei 103266Lr, 104267Rf, 105266‑268Db, 111281Rg, and 112282Cn occurring as end products of these α-decay chains. The behavior of fragment mass distribution and competitive emergence of the dominant decay mode, i.e., the α-emission versus spontaneous fission (SF), are studied for identifying the most probable heavy fission fragments, along with the estimation of SF half-life times T1/2SF and total kinetic energy (TKE) of the above noted isotopes of Z = 103-112 nuclei decaying via the SF process. The mass distributions of chosen nuclei are clearly symmetric, independent of mass and temperature. The most preferred decay fragment is found to lie in the neighborhood of doubly magic shell closures of Z = 50 and N = 82, with largest preformation factor P0. In addition, a comparative study of the “hot compact” and “cold elongated” configurations of β2i-deformed and 𝜃iopt-oriented nuclei indicates significantly different behaviors of the two mass fragmentation yields, favoring “hot compact” configuration.

Cement As a Waste Form for Nuclear Fission Products: The Case of 90Sr and Its Daughters [Cement As a Container for Nuclear Fission Products: The Case of 90Sr and Its Daughters

DOE PAGES

Dezerald, Lucile; Kohanoff, Jorge J.; Correa, Alfredo A.; ...

2015-10-29

One of the main challenges faced by the nuclear industry is the long-term confinement of nuclear waste. Because it is inexpensive and easy to manufacture, cement is the material of choice to store large volumes of radioactive materials, in particular the low-level medium-lived fission products. It is therefore of utmost importance to assess the chemical and structural stability of cement containing radioactive species. Here, we use ab initio calculations based on density functional theory (DFT) to study the effects of 90Sr insertion and decay in C–S–H (calcium-silicate-hydrate) in order to test the ability of cement to trap and hold thismore » radioactive fission product and to investigate the consequences of its β-decay on the cement paste structure. We show that 90Sr is stable when it substitutes the Ca 2+ ions in C–S–H, and so is its daughter nucleus 90Y after β-decay. Interestingly, 90Zr, daughter of 90Y and final product in the decay sequence, is found to be unstable compared to the bulk phase of the element at zero K but stable when compared to the solvated ion in water. Furthermore, cement appears as a suitable waste form for 90Sr storage.« less

Acceleration of Singlet Fission in an Aza-Derivative of TIPS-Pentacene.

PubMed

Herz, Julia; Buckup, Tiago; Paulus, Fabian; Engelhart, Jens; Bunz, Uwe H F; Motzkus, Marcus

2014-07-17

The influence of the carbon to nitrogen substitution on the photoinduced dynamics of TIPS-pentacene was investigated by ultrafast transient absorption measurements on spin-coated thin films in the visible and in the near-infrared spectral region. A global target analysis was performed to provide a detailed picture of the excited-state dynamics. We found that the chemical modification has a high impact on the triplet formation and leads to shorter dynamics; hence it speeds up the singlet fission process. A faster relaxation from the singlet into the triplet manifold implies a higher efficiency because other relaxation channels are avoided. The air-stable aza-derivatives have the potential to exceed the energy conversion efficiency of TIPS-pentacene.

Non-gravitational force modeling of Comet 81P/Wild 2. II. Rotational evolution

NASA Astrophysics Data System (ADS)

Gutiérrez, Pedro J.; Davidsson, Björn J. R.

2007-11-01

In this paper, we have studied both the dynamical and the rotational evolution of an 81P/Wild 2-like comet under the effects of the outgassing-induced force and torque. The main aim is to study if it is possible to reproduce the non-gravitational orbital changes observed in this comet, and to establish the likely evolution of both orbital and rotational parameters. To perform this study, a simple thermophysical model has been used to estimate the torque acting on the nucleus. Once the torque is calculated, Euler equations are solved numerically considering a nucleus mass directly estimated from the changes in the orbital elements (as determined from astrometry). According to these simulations, when the water production rate and changes in orbital parameters for 1997, as well as observational rotational parameters for 2004 are imposed as constraints, the change in the orbital period of 81P/Wild 2, ΔP=P˙, will decrease so that P¨=-5 to -1minorbit, which is similar to the actual tendency observed from 1988 up to 1997. This nearly constant decreasing can be explained as due to a slight drift of the spin axis orientation towards larger ecliptic longitudes. After studying the possible spin axis orientations proposed for 1997, simulations suggest that the spin obliquity and argument (I,Φ)=(56°,167°) is the most likely. As for rotational evolution, changes per orbit smaller than 10% of the actual spin velocity are probable, while the most likely value corresponds to a change between 2 and 7% of the spin velocity. Equally, net changes in the spin axis orientation of 4°-8° per orbit are highly expected.

Projected Shell Model Description of Positive Parity Band of 130Pr Nucleus

NASA Astrophysics Data System (ADS)

Singh, Suram; Kumar, Amit; Singh, Dhanvir; Sharma, Chetan; Bharti, Arun; Bhat, G. H.; Sheikh, J. A.

2018-02-01

Theoretical investigation of positive parity yrast band of odd-odd 130Pr nucleus is performed by applying the projected shell model. The present study is undertaken to investigate and verify the very recently observed side band in 130Pr theoretically in terms of quasi-particle (qp) configuration. From the analysis of band diagram, the yrast as well as side band are found to arise from two-qp configuration πh 11/2 ⊗ νh 11/2. The present calculations are viewed to have qualitatively reproduced the known experimental data for yrast states, transition energies, and B( M1) / B( E2) ratios of this nucleus. The recently observed positive parity side band is also reproduced by the present calculations. The energy states of the side band are predicted up to spin 25+, which is far above the known experimental spin of 18+ and this could serve as a motivational factor for future experiments. In addition, the reduced transition probability B( E2) for interband transitions has also been calculated for the first time in projected shell model, which would serve as an encouragement for other research groups in the future.

K-mixing in the doubly mid-shell nuclide 170Dy and the role of vibrational degeneracy

NASA Astrophysics Data System (ADS)

Söderström, P.-A.; Walker, P. M.; Wu, J.; Liu, H. L.; Regan, P. H.; Watanabe, H.; Doornenbal, P.; Korkulu, Z.; Lee, P.; Liu, J. J.; Lorusso, G.; Nishimura, S.; Phong, V. H.; Sumikama, T.; Xu, F. R.; Yagi, A.; Zhang, G. X.; Ahn, D. S.; Alharbi, T.; Baba, H.; Browne, F.; Bruce, A. M.; Carroll, R. J.; Chae, K. Y.; Dombradi, Zs.; Estrade, A.; Fukuda, N.; Griffin, C. J.; Ideguchi, E.; Inabe, N.; Isobe, T.; Kanaoka, H.; Kanaya, S.; Kojouharov, I.; Kondev, F. G.; Kubo, T.; Kubono, S.; Kurz, N.; Kuti, I.; Lalkovski, S.; Lane, G. J.; Lee, E. J.; Lee, C. S.; Lotay, G.; Moon, C.-B.; Nishizuka, I.; Niţă, C. R.; Odahara, A.; Patel, Z.; Podolyák, Zs.; Roberts, O. J.; Sakurai, H.; Schaffner, H.; Shand, C. M.; Suzuki, H.; Takeda, H.; Terashima, S.; Vajta, Zs.; Valiente-Dòbon, J. J.; Xu, Z. Y.

2016-11-01

A detailed study of the structure of the doubly mid-shell nucleus 104 1 66 170 Dy has been carried out, following isomeric and β decay. We have measured the yrast band up to the spin-parity Jπ =6+ state, the K = 2γ-vibration band up to the 5+ state, a low-lying negative-parity band based on a 2- state that could be a candidate for the lowest energy octupole vibration state within this nucleus, and a candidate for the Kπ =6+ two quasi-particle isomer. This state was determined to have an excitation energy of 1643.91(23) keV and a half life of 0.99(4) μs, with a reduced hindrance for its decay to the ground-state band an order of magnitude lower than predicted by NpNn systematics. This is interpreted as being due to γ-vibrational mixing from a near degeneracy of the isomer and the 6+ state of the γ band. Furthermore, the parent nucleus 170Tb has been determined to have a half-life of 0.91 (+18-13) s with a possible spin-parity of 2-.

On the Nature of the Cherdyntsev-Chalov Effect

NASA Astrophysics Data System (ADS)

Timashev, S. F.

2018-06-01

It is shown that the Cherdyntsev-Chalov effect, usually presented as the separation of even isotopes of uranium upon their transition from the solid to the liquid phase, can include initiated acceleration of the radioactive decay of uranium-238 nuclei during the formation of cracks in geologically (seismic and volcanically) active zones of the Earth's crust. The fissuring of the solid-phase medium leads to an increase in mechanical tensile stress and the emergence of strong local electric fields, resulting in the injection of chemical-scale high-energy electrons into the aqueous phase of the cracks. Under these conditions, the e - catalytic decay of uranium-238 nucleus studied earlier can occur during the formation of metastable protactinium-238 nuclei with locally distorted nucleon structure, which subequently undergo β-decay with the formation of thorium-234 and helium-4 nuclei as products of the fission of the initial uranium-238 nucleus with a characteristic period of several years. The observed increased activity of uranium-234 nuclei that form during the subsequent β-decay of thorium and then protactinium is associated with the initiated fission of uranium-238. The possibility is discussed of developing thermal power by using existing wastes from uranium production that contain uranium-238 to activate this isotope through the mechanochemical processing of these wastes in aqueous media with the formation of 91 238 Pa isu , the half-life of which is several years.

Lifetime measurements in N=Z 72Kr

NASA Astrophysics Data System (ADS)

Andreoiu, C.; Svensson, C. E.; Austin, R. A. E.; Carpenter, M. P.; Dashdorj, D.; Finlay, P.; Freeman, S. J.; Garrett, P. E.; Görgen, A.; Greene, J.; Grinyer, G. F.; Hyland, B.; Jenkins, D.; Johnston-Theasby, F.; Joshi, P.; Machiavelli, A. O.; Moore, F.; Mukherjee, G.; Phillips, A. A.; Reviol, W.; Sarantites, D. G.; Schumaker, M. A.; Seweryniak, D.; Smith, M. B.; Valiente-Dobón, J. J.; Wadsworth, R.

2006-07-01

High-spin states in the N=Z nucleus 72Kr have been populated in the 40Ca(40Ca, 2α)72Kr fusion-evaporation reaction at a beam energy of 165 MeV and using a thin isotopically enriched 40Ca target. The experiment, performed at Argonne National Laboratory close to Chicago, USA, employed the Gammasphere array for γ-ray detection coupled to the Microball array for charged particle detection. The previously observed bands in 72Kr were extended to a higher excitation energy of ~24 MeV and higher angular momentum of 30planck. Using the Doppler-shift attenuation method, the lifetimes of high-spin states were measured for the first time in order to investigate deformation changes associated with the g9/2 proton and neutron alignments in this N=Z nucleus. An excellent agreement with theoretical calculations including only standard t=1 np pairing was observed.

Skyrme density functional description of the double magic 78Ni nucleus

NASA Astrophysics Data System (ADS)

Brink, D. M.; Stancu, Fl.

2018-06-01

We calculate the single-particle spectrum of the double magic nucleus 78Ni in a Hartree-Fock approach using the Skyrme density-dependent effective interaction containing central, spin-orbit, and tensor parts. We show that the tensor part has an important effect on the spin-orbit splitting of the proton 1 f orbit that may explain the survival of magicity so far from the stability valley. We confirm the inversion of the 1 f 5 /2 and 2 p 3 /2 levels at the neutron number 48 in the Ni isotopic chain expected from previous Monte Carlo shell-model calculations and supported by experimental observation.

Singularities in the lineshape of a second-order perturbed quadrupolar nucleus. The magic-angle spinning case.

PubMed

Field, Timothy R; Bain, Alex D

2014-01-01

For a nucleus with a half-integral spin and a strong quadrupole coupling, the central transition (from magnetic quantum number -1/2 to +1/2) in the spectrum shows a characteristic lineshape. By strong coupling, we mean an interaction strong enough so that second-order perturbation theory is needed, yet still sufficient. The spectrum of a static sample is well-known and the magic-angle-spinning (MAS spectrum) is different, but still can be calculated. The important features of both these spectra are singularities and steps in the lineshape, since these are the main tools in fitting the calculated spectrum to experimental data. A useful tool in this investigation is a plot of the frequency as a function of orientation over the surface of the unit sphere. These plots have maxima, minima and saddle points, and these correspond to the features of the spectrum. We used these plots to define both the positions and derive new formulae for the heights of the features and we now extend this to the magic-angle spinning case. For the first time, we identify the orientations corresponding to the features of the MAS spectra and derive formulae for the heights. We then compare the static and MAS cases and show the relationships between the features in the two spectra. Copyright © 2014 Elsevier Inc. All rights reserved.

General Description of Fission Observables: GEF Model Code

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schmidt, K.-H.; Jurado, B., E-mail: jurado@cenbg.in2p3.fr; Amouroux, C.

2016-01-15

The GEF (“GEneral description of Fission observables”) model code is documented. It describes the observables for spontaneous fission, neutron-induced fission and, more generally, for fission of a compound nucleus from any other entrance channel, with given excitation energy and angular momentum. The GEF model is applicable for a wide range of isotopes from Z = 80 to Z = 112 and beyond, up to excitation energies of about 100 MeV. The results of the GEF model are compared with fission barriers, fission probabilities, fission-fragment mass- and nuclide distributions, isomeric ratios, total kinetic energies, and prompt-neutron and prompt-gamma yields and energymore » spectra from neutron-induced and spontaneous fission. Derived properties of delayed neutrons and decay heat are also considered. The GEF model is based on a general approach to nuclear fission that explains a great part of the complex appearance of fission observables on the basis of fundamental laws of physics and general properties of microscopic systems and mathematical objects. The topographic theorem is used to estimate the fission-barrier heights from theoretical macroscopic saddle-point and ground-state masses and experimental ground-state masses. Motivated by the theoretically predicted early localisation of nucleonic wave functions in a necked-in shape, the properties of the relevant fragment shells are extracted. These are used to determine the depths and the widths of the fission valleys corresponding to the different fission channels and to describe the fission-fragment distributions and deformations at scission by a statistical approach. A modified composite nuclear-level-density formula is proposed. It respects some features in the superfluid regime that are in accordance with new experimental findings and with theoretical expectations. These are a constant-temperature behaviour that is consistent with a considerably increased heat capacity and an increased pairing condensation energy that is consistent with the collective enhancement of the level density. The exchange of excitation energy and nucleons between the nascent fragments on the way from saddle to scission is estimated according to statistical mechanics. As a result, excitation energy and unpaired nucleons are predominantly transferred to the heavy fragment in the superfluid regime. This description reproduces some rather peculiar observed features of the prompt-neutron multiplicities and of the even-odd effect in fission-fragment Z distributions. For completeness, some conventional descriptions are used for calculating pre-equilibrium emission, fission probabilities and statistical emission of neutrons and gamma radiation from the excited fragments. Preference is given to simple models that can also be applied to exotic nuclei compared to more sophisticated models that need precise empirical input of nuclear properties, e.g. spectroscopic information. The approach reveals a high degree of regularity and provides a considerable insight into the physics of the fission process. Fission observables can be calculated with a precision that complies with the needs for applications in nuclear technology without specific adjustments to measured data of individual systems. The GEF executable runs out of the box with no need for entering any empirical data. This unique feature is of valuable importance, because the number of systems and energies of potential significance for fundamental and applied science will never be possible to be measured. The relevance of the approach for examining the consistency of experimental results and for evaluating nuclear data is demonstrated.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gurgi, L. A.; Regan, P. H.; Söderström, P. -A.

In-flight fission of a 345 MeV per nucleon 238U primary beam on a 2 mm thick 9Be target has been used to produce and study the decays of a range of neutron-rich nuclei centred around the doubly mid-shell nucleus 170Dy at the RIBF Facility, RIKEN, Japan. The produced secondary fragments of interest were identified event-by-event using the BigRIPS separator. The fragments were implanted into the WAS3ABI position sensitive silicon active stopper which allowed pixelated correlations between implants and their subsequent β-decay. Discrete γ-ray transitions emitted following decays from either metastable states or excited states populated following beta decay were identifiedmore » using the 84 coaxial high-purity germanium (HPGe) detectors of the EURICA spectrometer, which was complemented by 18 additional cerium-doped lanthanum bromide (LaBr3) fast-timing scintillation detectors from the FATIMA collaboration. This paper presents the internal decay of a metastable isomeric excited state in the odd-odd nucleus 168Tb, which corresponds to a single proton-neutron hole configuration in the valence maximum nucleus 170Dy. These data represent the first information on excited states in this nucleus, which is the most neutron-rich odd-odd isotope of terbium (Z=65) studied to date. Nilsson configurations associated with an axially symmetric, prolate-deformed nucleus are proposed for the 168Tb ground state the observed isomeric state by comparison with Blocked BCS-Nilsson calculations.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gurgi, L. A.; Regan, P. H.; Söderström, P. -A.

In-flight fission of a 345 MeV per nucleon 238U primary beam on a 2 mm thick 9Be target has been used to produce and study the decays of a range of neutron-rich nuclei centred around the doubly mid-shell nucleus 170Dy at the RIBF Facility, RIKEN, Japan. The produced secondary fragments of interest were identified event-by-event using the BigRIPS separator. The fragments were implanted into the WAS3ABI position sensitive silicon active stopper which allowed pixelated correlations between implants and their subsequent β-decay. Discrete γ-ray transitions emitted following decays from either metastable states or excited states populated following beta decay were identifiedmore » using the 84 coaxial high-purity germanium (HPGe) detectors of the EURICA spectrometer, which was complemented by 18 additional cerium-doped lanthanum bromide (LaBr 3) fast-timing scintillation detectors from the FATIMA collaboration. This paper presents the internal decay of a metastable isomeric excited state in the odd-odd nucleus 168Tb, which corresponds to a single proton-neutron hole configuration in the valence maximum nucleus 170Dy. These data represent the first information on excited states in this nucleus, which is the most neutron-rich odd-odd isotope of terbium (Z = 65) studied to date. Here, Nilsson configurations associated with an axially symmetric, prolate-deformed nucleus are proposed for the 168Tb ground state the observed isomeric state by comparison with Blocked BCS-Nilsson calculations.« less

Processes in massive nuclei reactions and the way to complete fusion of reactants. What perspectives for the synthesis of heavier superheavy elements?

NASA Astrophysics Data System (ADS)

Mandaglio, G.; Nasirov, A. K.; Curciarello, F.; De Leo, V.; Romaniuk, M.; Fazio, G.; Giardina, G.

2012-12-01

By using the dinuclear system (DNS) model we determine the capture of reactants at the first stage of reaction, the competition between the DNS decay by the quasifission (QF) and the complete fusion (CF) process up to formation of the compound nucleus (CN) having compact shape. Further evolution of the CN is considered as its fission into two fragments or formation of evaporation residues (ER) by its cooling after emission of neutrons or/and charged light particles. Disappearance of the CN fission barrier due to its fast rotation leads to the fast fission (FF) by formation of fissionlike fragments. The results of calculations for the mass symmetric 136Xe+136Xe reaction, almost mass symmetric 108Mo+144Ba reaction, and mass asymmetric like 24Mg+238U and 34S+248Cm reactions are discussed. The fusion probability PCN calculated for many massive nuclei reactions leading to formation of superheavy nuclei have been analyzed. The reactions which can lead in perspective to the synthesis of superheavy elements in the Z = 120 - 126 range and, eventually, also to heaviest nuclei, are discussed.

High-spin spectroscopy of 139Ce

NASA Astrophysics Data System (ADS)

Kaim, S.; Petrache, C. M.; Gargano, A.; Itaco, N.; Zerrouki, T.; Leguillon, R.; Astier, A.; Deloncle, I.; Konstantinopoulos, T.; Régis, J. M.; Wilmsen, D.; Melon, B.; Nannini, A.; Ducoin, C.; Guinet, D.; Bhattacharjee, T.

2015-02-01

High-spin states in 139Ce have been populated using the 130Te(14C,5 n ) reaction. The level scheme has been extended to higher spins, including a new band of dipole transitions. The parity of several states has been changed from negative to positive, mainly based on the comparison with the level structure of the core nucleus 140Ce and the results of a realistic shell-model calculation. The dipole band is interpreted as a magnetic rotation band with π h11/2 2⊗ν h11/2 -1 configuration built on small deformation axial shape with (ɛ2=0.12 ,γ =0∘) .

All possible tripartitions of {}(236) 236U isotope in collinear configuration

NASA Astrophysics Data System (ADS)

Santhosh, K. P.; Krishnan, Sreejith; Joseph, Jayesh George

2018-07-01

Using the recently proposed unified ternary fission model (UTFM), the tripartition of ^{236}U isotope was studied for all possible fragmentations, in which the interacting potential barrier is taken as the sum of the Coulomb and proximity potentials with fragments in collinear configuration. The highest yield is obtained for the fragmentation ^{48}Ca{+}^{58}Ti{+}^{130}Sn and next highest yield is found for ^{58}Cr{+}^{46}Ar{+}^{132}Sn, which stress the importance of doubly magic or near doubly magic nuclei in the tripartition of ^{236}U isotope. The formation of ^{68}Ni and ^{70}Ni as the edge fragments linking the doubly magic nucleus ^{132}Sn by the isotope of Si is in good agreement with experimental and theoretical studies, in the collinear cluster tripartition of ^{236}U isotope which reveals the reliability of our model (UTFM) in ternary fission.

Fission yeast APC/C activators Slp1 and Fzr1 sequentially trigger two consecutive nuclear divisions during meiosis.

PubMed

Chikashige, Yuji; Yamane, Miho; Okamasa, Kasumi; Osakada, Hiroko; Tsutsumi, Chihiro; Nagahama, Yuki; Fukuta, Noriko; Haraguchi, Tokuko; Hiraoka, Yasushi

2017-04-01

In meiosis, two rounds of nuclear division occur consecutively without DNA replication between the divisions. We isolated a fission yeast mutant in which the nucleus divides only once to generate two spores, as opposed to four, in meiosis. In this mutant, we found that the initiation codon of the slp1 + gene is converted to ATA, producing a reduced amount of Slp1. As a member of the Fizzy family of anaphase-promoting complex/cyclosome (APC/C) activators, Slp1 is essential for vegetative growth; however, the mutant allele shows a phenotype only in meiosis. Slp1 insufficiency delays degradation of maturation-promoting factor at the first meiotic division, and another APC/C activator, Fzr1, which acts late in meiosis, terminates meiosis immediately after the delayed first division to produce two viable spores. © 2017 Federation of European Biochemical Societies.

In-beam fissio study at JAEA for heavy element synthesis

NASA Astrophysics Data System (ADS)

Nishio, K.; Ikezoe, H.; Hofmann, S.; Ackermann, D.; Aritomo, Y.; Comas, V. F.; Düllmann, Ch. E.; Heinz, S.; Heredia, J. A.; Heßberger, F. P.; Hirose, K.; Khuyagbaatar, J.; Kindler, B.; Kojouharov, I.; Lommel, B.; Makii, M.; Mann, R.; Mitsuoka, S.; Nishinaka, I.; Ohtsuki, T.; Saro, S.; Schädel, M.; Popeko, A. G.; Türler, A.; Wakabayashi, Y.; Watanabe, Y.; Yakushev, A.; Yeremin, A.

2013-04-01

Fission fragment mass distributions were measured in the heavy-ion induced fission using 238U target nucleus. The mass distributions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and qasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their incident energy dependence. Fusion probability was determined in the analysis. Evaporation residue cross sections were calculated with a statistical model in the reactions of 30Si+238U and 34S+238U using the obtained fusion probability in the entrance channel. The results agree with the measured cross sections of 263,264Sg and 267,268Hs, produced by 30Si+238U and 34S+238U, respectively. It is also suggested that the sub-barrier energies can be used for heavy element synthesis.

Femtosecond stimulated Raman evidence for charge-transfer character in pentacene singlet fission† †Electronic supplementary information (ESI) available: Actinic pump spectrum, discussion on ground state addition process, peak fitting procedure, transient absorption data, power dependence measurements, etalon pulse shaping, TIPS-pentacene FSRS data, and optimized geometry and frequency calculation results. See DOI: 10.1039/c7sc03496b

PubMed Central

Hart, Stephanie M.; Silva, W. Ruchira

2017-01-01

Singlet fission is a spin-allowed process in which an excited singlet state evolves into two triplet states. We use femtosecond stimulated Raman spectroscopy, an ultrafast vibrational technique, to follow the molecular structural evolution during singlet fission in order to determine the mechanism of this process. In crystalline pentacene, we observe the formation of an intermediate characterized by pairs of excited state peaks that are red- and blue-shifted relative to the ground state features. We hypothesize that these features arise from the formation of cationic and anionic species due to partial transfer of electron density from one pentacene molecule to a neighboring molecule. These observations provide experimental evidence for the role of states with significant charge-transfer character which facilitate the singlet fission process in pentacene. Our work both provides new insight into the singlet fission mechanism in pentacene and demonstrates the utility of structurally-sensitive time-resolved spectroscopic techniques in monitoring ultrafast processes. PMID:29675170

Do Gluons Carry Proton Spin? - Toward Resolving the Spin Crisis (445th Brookhaven Lecture)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bazilevsky, Alexander

2009-01-21

Just as Earth and other planets spin within the solar system, subatomic quark and gluon particles spin within the protons and neutrons that spin within the nucleus of an atom. Quantum Chromodynamics (QCD) is a theory that describes interactions between subatomic particles and it has played a defining role in understanding the spin of protons and neutrons, which make up most of the visible mass in the universe. Experiments first completed at CERN and furthered at several other laboratories around the world revealed that surprisingly, quarks and their partnering anti-quarks are responsible for only 20 to 30 percent of protonmore » spin. These findings pointed to what would become known as "spin crisis." More recent experiments at BNL's Relativistic Heavy Ion Collider (RHIC), the first collider to smash protons that are "polarized," or made to spin in the same orientation, have helped to isolate the role of the gluon's spin within the spinning proton in hopes of resolving this crisis. In his lecture, Bazilevsky will explain how data from RHIC's PHENIX and STAR detectors help to reveal the role of gluons in the proton's spin. Bazilevsky will also discuss long- and short-term plans to attain a deeper look into the proton spin structure, utilizing RHIC and its future upgrades« less

Electron Spin Resonance (ESR) studies of returned comet nucleus samples

NASA Technical Reports Server (NTRS)

Tsay, Fun-Dow; Kim, Soon Sam; Liang, Ranty H.

1989-01-01

The most important objective of the Comet Nucleus Sample Returm Mission is to return samples which could reflect formation conditions and evolutionary processes in the early solar nebula. It is expected that the returned samples will consist of fine-grained silicate materials mixed with ices composed of simple molecules such as H2O, NH3, CH4 as well as organics and/or more complex compounds. Because of the exposure to ionizing radiation from cosmic-ray, gamma-ray, and solar wind protons at low temperature, free radicals are expected to be formed and trapped in the solid ice matrices. The kind of trapped radical species together with their concentration and thermal stability can be used as a dosimeter as well as a geothermometer to determine thermal and radiation histories as well as outgassing and other possible alternation effects since the nucleus material was formed. Since free radicals that are known to contain unpaired electrons are all paramagnetic in nature, they can be readily detected and characterized in their native form by the Electron Spin Resonance (ESR) method. In fact, ESR has been shown to be a non-destructive, highly sensitive tool for the detection and characterization of paramagnetic, ferromagnetic, and radiation damage centers in terrestrial and extraterrestrial geological samples. The potential use of ESR as an effective method in the study of returned comet nucleus samples, in particular, in the analysis of fine-grained solid state icy samples is discussed.

The study of the physics of cometary nuclei

NASA Technical Reports Server (NTRS)

Whipple, F. L.

1984-01-01

The observations of comet P/Holmes 1892III, exhibiting two 8 to 10 magnitude bursts, were carefully analyzed. The phenomena are consistent with the grazing encounter of a small satellite with the nucleus. The grazing encounter produced, besides the first great burst, an active area on the nucleus, which was rotating retrograde with a period of 16.3 hr and inclination nearly 180 deg. After the final encounter, the spin period was essentially unchanged, but two areas became active, separated some 164 deg in longitude on the nucleus. After the first burst the total magnitude fell less than two magnitudes, while the nuclear region remained diffuse or complex, rarely if ever showing a stellar appearance. The fading was much more rapid after the second burst (barely naked eye at maximum) while the nucleus frequently stellar after the first day. It seems reasonable to conclude that the grazing encounter distributed a volume of large chunks in the neighborhood of the nucleus, maintaining activity for weeks.

First spin-resolved electron distributions in crystals from combined polarized neutron and X-ray diffraction experiments.

PubMed

Deutsch, Maxime; Gillon, Béatrice; Claiser, Nicolas; Gillet, Jean-Michel; Lecomte, Claude; Souhassou, Mohamed

2014-05-01

Since the 1980s it has been possible to probe crystallized matter, thanks to X-ray or neutron scattering techniques, to obtain an accurate charge density or spin distribution at the atomic scale. Despite the description of the same physical quantity (electron density) and tremendous development of sources, detectors, data treatment software etc., these different techniques evolved separately with one model per experiment. However, a breakthrough was recently made by the development of a common model in order to combine information coming from all these different experiments. Here we report the first experimental determination of spin-resolved electron density obtained by a combined treatment of X-ray, neutron and polarized neutron diffraction data. These experimental spin up and spin down densities compare very well with density functional theory (DFT) calculations and also confirm a theoretical prediction made in 1985 which claims that majority spin electrons should have a more contracted distribution around the nucleus than minority spin electrons. Topological analysis of the resulting experimental spin-resolved electron density is also briefly discussed.

Can the waiting-point nucleus 78Ni be studied at an on-line mass-separator?

NASA Astrophysics Data System (ADS)

Wöhr, A.; Andreyev, A.; Bijnens, N.; Breitenbach, J.; Franchoo, S.; Huyse, M.; Kudryavtsev, Y. A.; Piechaczek, A.; Raabe, R. R.; Reusen, I.; Vermeeren, L.; Van Duppen, P.

1997-02-01

Short-lived nickel isotopes have been studied using a chemically selective Ion Guide Laser Ion Source (IGLIS) based on resonance ionisation of atoms at the Leuven Isotope Separator On-Line (LISOL) separator. The decay properties of different Ni isotopes have been studied using β-γ-coincidences. Experimental production rates of proton induced fission of 238U are obtained for 69,71Ni. These numbers are in a strong disagreement with Silberg-Tsao calculations.

Monte Carlo based dosimetry for neutron capture therapy of brain tumors

NASA Astrophysics Data System (ADS)

Zaidi, Lilia; Belgaid, Mohamed; Khelifi, Rachid

2016-11-01

Boron Neutron Capture Therapy (BNCT) is a biologically targeted, radiation therapy for cancer which combines neutron irradiation with a tumor targeting agent labeled with a boron10 having a high thermal neutron capture cross section. The tumor area is subjected to the neutron irradiation. After a thermal neutron capture, the excited 11B nucleus fissions into an alpha particle and lithium recoil nucleus. The high Linear Energy Transfer (LET) emitted particles deposit their energy in a range of about 10μm, which is of the same order of cell diameter [1], at the same time other reactions due to neutron activation with body component are produced. In-phantom measurement of physical dose distribution is very important for BNCT planning validation. Determination of total absorbed dose requires complex calculations which were carried out using the Monte Carlo MCNP code [2].

In-beam spectroscopy of medium- and high-spin states in Ce 133

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ayangeakaa, A. D.; Garg, U.; Petrache, C. M.

2016-05-01

Medium and high-spin states in Ce-133 were investigated using the Cd-116(Ne-22, 5n) reaction and the Gammasphere array. The level scheme was extended up to an excitation energy of similar to 22.8 MeV and spin 93/2 (h) over bar. Eleven bands of quadrupole transitions and two new dipole bands are identified. The connections to low-lying states of the previously known, high-spin triaxial bands were firmly established, thus fixing the excitation energy and, in many cases, the spin parity of the levels. Based on comparisons with cranked Nilsson-Strutinsky calculations and tilted axis cranking covariant density functional theory, it is shown that allmore » observed bands are characterized by pronounced triaxiality. Competing multiquasiparticle configurations are found to contribute to a rich variety of collective phenomena in this nucleus.« less

The Transuranium Elements: Early History (Nobel Lecture)

DOE R&D Accomplishments Database

McMillan, E. M.

1951-12-12

In this talk the author tells of the circumstances that led to the discovery of neptunium, the first element beyond uranium, and the partial identification of plutonium, the next one beyond that. The part of the story that lies before 1939 has already been recounted here in the Nobel lectures of Fermi and Hahn. Rather the author starts with the discovery of fission by Hahn and Strassmann. News of this momentous discovery reached Berkeley early in 1939. The staff of the Radiation Laboratory was put into a state of great excitement and several experiments of a nature designed to check and extend the announced results were started, using ionization chambers and pulse amplifiers, cloud chambers, chemical methods, and so forth. The author decided to do an experiment of a very simple kind. When a nucleus of uranium absorbs a neutron and fission takes place, the two resulting fragments fly apart with great violence, sufficient to propel them through air or other matter for some distance. This distance, called the "range", is quantity of some interest, and the author undertook to measure it by observing the depth of penetration of the fission fragments in a stack of thin aluminum foils. The fission fragments came from a thin layer of uranium oxide spread on a sheet of paper, and exposed to neutrons from a beryllium target bombarded by 8 Mev deuterons in the 37-inch cyclotron. The aluminum foils, each with a thickness of about half a milligram per square centimeter, were stacked like the pages of a book in immediate contact with the layer of uranium oxide. After exposure to the neutrons, the sheets of aluminum were separated and examined for radioactivity by means of an ionization chamber. The fission fragments of course are radioactive atoms, and their activity is found where they stop.

Sensitivity Analysis of Cf-252 (sf) Neutron and Gamma Observables in CGMF

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carter, Austin Lewis; Talou, Patrick; Stetcu, Ionel

CGMF is a Monte Carlo code that simulates the decay of primary fission fragments by emission of neutrons and gamma rays, according to the Hauser-Feshbach equations. As the CGMF code was recently integrated into the MCNP6.2 transport code, great emphasis has been placed on providing optimal parameters to CGMF such that many different observables are accurately represented. Of these observables, the prompt neutron spectrum, prompt neutron multiplicity, prompt gamma spectrum, and prompt gamma multiplicity are crucial for accurate transport simulations of criticality and nonproliferation applications. This contribution to the ongoing efforts to improve CGMF presents a study of the sensitivitymore » of various neutron and gamma observables to several input parameters for Californium-252 spontaneous fission. Among the most influential parameters are those that affect the input yield distributions in fragment mass and total kinetic energy (TKE). A new scheme for representing Y(A,TKE) was implemented in CGMF using three fission modes, S1, S2 and SL. The sensitivity profiles were calculated for 17 total parameters, which show that the neutron multiplicity distribution is strongly affected by the TKE distribution of the fragments. The total excitation energy (TXE) of the fragments is shared according to a parameter RT, which is defined as the ratio of the light to heavy initial temperatures. The sensitivity profile of the neutron multiplicity shows a second order effect of RT on the mean neutron multiplicity. A final sensitivity profile was produced for the parameter alpha, which affects the spin of the fragments. Higher values of alpha lead to higher fragment spins, which inhibit the emission of neutrons. Understanding the sensitivity of the prompt neutron and gamma observables to the many CGMF input parameters provides a platform for the optimization of these parameters.« less

Rotational Failure of Rubble-pile Bodies: Influences of Shear and Cohesive Strengths

NASA Astrophysics Data System (ADS)

Zhang, Yun; Richardson, Derek C.; Barnouin, Olivier S.; Michel, Patrick; Schwartz, Stephen R.; Ballouz, Ronald-Louis

2018-04-01

The shear and cohesive strengths of a rubble-pile asteroid could influence the critical spin at which the body fails and its subsequent evolution. We present results using a soft-sphere discrete element method to explore the mechanical properties and dynamical behaviors of self-gravitating rubble piles experiencing increasing rotational centrifugal forces. A comprehensive contact model incorporating translational and rotational friction and van der Waals cohesive interactions is developed to simulate rubble-pile asteroids. It is observed that the critical spin depends strongly on both the frictional and cohesive forces between particles in contact; however, the failure behaviors only show dependence on the cohesive force. As cohesion increases, the deformation of the simulated body prior to disruption is diminished, the disruption process is more abrupt, and the component size of the fissioned material is increased. When the cohesive strength is high enough, the body can disaggregate into similar-size fragments, which could be a plausible mechanism to form asteroid pairs or active asteroids. The size distribution and velocity dispersion of the fragments in high-cohesion simulations show similarities to the disintegrating asteroid P/2013 R3, indicating that this asteroid may possess comparable cohesion in its structure and experience rotational fission in a similar manner. Additionally, we propose a method for estimating a rubble pile’s friction angle and bulk cohesion from spin-up numerical experiments, which provides the opportunity for making quantitative comparisons with continuum theory. The results show that the present technique has great potential for predicting the behaviors and estimating the material strengths of cohesive rubble-pile asteroids.

Calculated fission-fragment yield systematics in the region 74 <=Z <= 94 and 90 <=N <= 150

DOE PAGES

Möller, Peter; Randrup, Jørgen

2015-04-01

Background: In the seminal experiment by Schmidt et al. [Nucl. Phys. A 665, 221 (2000)] in which fission-fragment charge distributions were obtained for 70 nuclides, asymmetric distributions were seen above nucleon number A ≈ 226 and symmetric ones below. Because asymmetric fission had often loosely been explained as a preference for the nucleus to always exploit the extra binding of fragments near ¹³²Sn it was assumed that all systems below A ≈ 226 would fission symmetrically because available isotopes do not have a proton-to-neutron Z/N ratio that allows division into fragments near ¹³²Sn. But the finding by Andreyev et al.more » [Phys. Rev. Lett. 105, 252502 (2010)] did not conform to this expectation because the compound system ¹⁸⁰Hg was shown to fission asymmetrically. It was suggested that this was a new type of asymmetric fission, because no strong shell effects occur for any possible fragment division. Purpose: We calculate a reference database for fission-fragment mass yields for a large region of the nuclear chart comprising 987 nuclides. A particular aim is to establish whether ¹⁸⁰Hg is part of a contiguous region of asymmetric fission, and if so, its extent, or if not, in contrast to the actinides, there are scattered smaller groups of nuclei that fission asymmetrically in this area of the nuclear chart. Methods: We use the by now well benchmarked Brownian shape-motion method and perform random walks on the previously calculated five-dimensional potential-energy surfaces. The calculated shell corrections are damped out with energy according to a prescription developed earlier. Results: We have obtained a theoretical reference database of fission-fragment mass yields for 987 nuclides. These results show an extended region of asymmetric fission with approximate extension 74 ≤ Z ≤ 85 and 100 ≤ N ≤ 120. The calculated yields are highly variable. We show 20 representative plots of these variable features and summarize the main aspects of our results in terms of “nuclear-chart” plots showing calculated degrees of asymmetry versus N and Z. Conclusions: Experimental data in this region are rare: only ten or so yield distributions have been measured, some with very limited statistics. We agree with several measurements with higher statistics. Regions where there might be differences between our calculated results and measurements lie near the calculated transition line between symmetric and asymmetric fission. To draw more definite conclusions about the accuracy of the present implementation of the Brownian shape-motion approach in this region experimental data, with reliable statistics, for a fair number of suitably located additional nuclides are clearly needed. Because the nuclear potential-energy structure is so different in this region compared to the actinide region, additional experimental data together with fission theory studies that incorporate additional, dynamical aspects should provide much new insight.« less

Magnetic resonance imaging of the subthalamic nucleus for deep brain stimulation.

PubMed

Chandran, Arjun S; Bynevelt, Michael; Lind, Christopher R P

2016-01-01

The subthalamic nucleus (STN) is one of the most important stereotactic targets in neurosurgery, and its accurate imaging is crucial. With improving MRI sequences there is impetus for direct targeting of the STN. High-quality, distortion-free images are paramount. Image reconstruction techniques appear to show the greatest promise in balancing the issue of geometrical distortion and STN edge detection. Existing spin echo- and susceptibility-based MRI sequences are compared with new image reconstruction methods. Quantitative susceptibility mapping is the most promising technique for stereotactic imaging of the STN.

Knockout of deuterons and tritons with large transverse momenta in pA collisions involving 50-GeV protons

NASA Astrophysics Data System (ADS)

Antonov, N. N.; Baldin, A. A.; Viktorov, V. A.; Gapienko, V. A.; Gapienko, G. S.; Gres', V. N.; Ilyushin, M. A.; Korotkov, V. A.; Mysnik, A. I.; Prudkoglyad, A. F.; Semak, A. A.; Terekhov, V. I.; Uglekov, V. Ya.; Ukhanov, M. N.; Chuiko, B. V.; Shimanskii, S. S.

2016-11-01

Formation of the d and t cumulative light nuclear fragments emitted from the nucleus with large transverse momenta at an angle of 35° in the laboratory frame is investigated. The data on collisions of 50-GeV protons with the C, Al, Cu, and W nuclei are collected using the extracted proton beam of the IHEP accelerator and the SPIN detector. The results indicate that the dominant contribution to formation of nuclear fragments comes from the local process of direct knockout from the nucleus.

Basic spin physics.

PubMed

Pipe, J G

1999-11-01

Magnetic resonance imaging is fundamentally a measurement of the magnetism inherent in some nuclear isotopes; of these the proton, or hydrogen atom, is of particular interest for clinical applications. The magnetism in each nucleus is often referred to as spin. A strong, static magnetic field B0 is used to align spins, forming a magnetic density within the patient. A second, rotating magnetic field B1 (RF pulse) is applied for a short duration, which rotates the spins away from B0 in a process called excitation. After the spins are rotated away from B0, the RF pulse is turned off, and the spins precess about B0. As long as the spins are all pointing in the same direction at any one time (have phase coherence), they act in concert to create rapidly oscillating magnetic fields. These fields in turn create a current in an appropriately placed receiver coil, in a manner similar to that of an electrical generator. The precessing magnetization decays rapidly in a duration roughly given by the T2 time constant. At the same time, but at a slower rate, magnetization forms again along the direction of B0; the duration of this process is roughly expressed by the T1 time constant. The precessional frequency of each spin is proportional to the magnetic field experienced at the nucleus. Small variations in this magnetic field can have dramatic effects on the MR image, caused in part by loss of phase coherence. These magnetic field variations can arise because of magnet design, the magnetic properties (susceptibility) of tissues and other materials, and the nuclear environment unique to various sites within any given molecule. The loss of phase coherence can be effectively eliminated by the use of RF refocusing pulses. Conventional MR imaging experiments can be characterized as either gradient echo or spin echo, the latter indicating the use of a RF refocusing pulse, and by the parameters TR, TE, and flip angle alpha. Tissues, in turn, are characterized by their individual spin density, M0, and by the T1, T2, and T2* time constants. Knowledge of these parameters allows one to calculate the resulting signal from a given tissue for a given MR imaging experiment.

K-mixing in the doubly mid-shell nuclide 170Dy and the role of vibrational degeneracy

DOE PAGES

Soderstrom, P. -A.; Walker, P. M.; Wu, J.; ...

2016-10-04

Here, a detailed study of the structure of the doubly mid-shell nucleus 170 66Dy 104 has been carried out, following isomeric and β decay. We have measured the yrast band up to the spin-parity J π = 6 + state, the K = 2 γ -vibration band up to the 5 + state, a low-lying negative-parity band based on a 2¯ state that could be a candidate for the lowest energy octupole vibration state within this nucleus, and a candidate for the K π = 6+ two quasi-particle isomer. This state was determined to have an excitation energy of 1643.91(23)more » keV and a half life of 0.99(4) μs, with a reduced hindrance for its decay to the groundstate band an order of magnitude lower than predicted by N pN n systematics. This is interpreted as being due to γ -vibrational mixing from a near degeneracy of the isomer and the 6 + state of the γ band. Furthermore, the parent nucleus 170Tb has been determined to have a half-life of 0.91( +18 –13) s with a possible spin-parity of 2¯.« less

Breit interaction effects in relativistic theory of the nuclear spin-rotation tensor.

PubMed

Aucar, I Agustín; Gómez, Sergio S; Giribet, Claudia G; Ruiz de Azúa, Martín C

2013-09-07

In this work, relativistic effects on the nuclear spin-rotation (SR) tensor originated in the electron-nucleus and electron-electron Breit interactions are analysed. To this end, four-component numerical calculations were carried out in model systems HX (X=H,F,Cl,Br,I). The electron-nucleus Breit interaction couples the electrons and nuclei dynamics giving rise to a purely relativistic contribution to the SR tensor. Its leading order in 1/c is of the same value as that of relativistic corrections on the usual second order expression of the SR tensor considered in previous work [I. A. Aucar, S. S. Gómez, J. I. Melo, C. G. Giribet, and M. C. Ruiz de Azúa, J. Chem. Phys. 138, 134107 (2013)], and therefore it is absolutely necessary to establish its relative importance. For the sake of completeness, the corresponding effect originating in the electron-electron Breit interaction is also considered. It is verified that in all cases these Breit interactions yield only very small corrections to the SR tensors of both the X and H nuclei in the present series of compounds. Results of the present work strongly suggest that in order to achieve experimental accuracy in the theoretical study of the SR tensor both electron-nucleus and electron-electron Breit effects can be safely neglected.

Lifetime measurements of high-lying short lived states in {sup 69}As

DOE Office of Scientific and Technical Information (OSTI.GOV)

Matejska-Minda, M.; Bednarczyk, P.; Fornal, B.

2012-10-20

Lifetimes of high-spin states in {sup 69}As have been measured using Doppler shift attenuation technique with the GASP and RFD setup. The determined transition probabilities indicate large deformation associated with some rotational bands in this nucleus.

Spin symmetry in the Dirac sea derived from the bare nucleon-nucleon interaction

NASA Astrophysics Data System (ADS)

Shen, Shihang; Liang, Haozhao; Meng, Jie; Ring, Peter; Zhang, Shuangquan

2018-06-01

The spin symmetry in the Dirac sea has been investigated with relativistic Brueckner-Hartree-Fock theory using the bare nucleon-nucleon interaction. Taking the nucleus 16O as an example and comparing the theoretical results with the data, the definition of the single-particle potential in the Dirac sea is studied in detail. It is found that if the single-particle states in the Dirac sea are treated as occupied states, the ground state properties are in better agreement with experimental data. Moreover, in this case, the spin symmetry in the Dirac sea is better conserved and it is more consistent with the findings using phenomenological relativistic density functionals.

SU-E-I-78: Neuromelanin in the Subthalamic Nucleus of Patients with Parkinson's Disease: An Electron Spin Resonance Spectroscopy Study.

PubMed

Gomez, J; Salmon, C Garrido; Filho, O Baffa; Santos, J Peixoto; Pitella, J

2012-06-01

Parkinson disease and related syndromes are associated directly with the concentrations of neuromelanin, iron and other heavy metals, and nowadays it is discussed the possible protective role of neuromelanin by the sequester redox active iron ions, reducing the formation of free hydroxyl radicals and therefore inactivating the iron ions that induce oxidative stress. The aim of this work is to study the concentration ratios between iron ions and neuromelanin in subthalamic nucleus of patients with Parkinson's disease (PD) using Electron Spin Resonance (ESR). Necropsy samples of subthalamic nucleus from eight human brains were studied: three non-affected by any neurodegenerative disease and five with Parkinson's disease. The samples were stored in formaldehyde and washed with a solution of 0.01 molar of ethylenediaminetetraacetic acid. ESR experiments were development in a JEOL FA-200 X-Band spectrometer at different temperatures between -170° C to room temperature. The relative concentrations of each species were estimated from the double integral values of the fitted spectra. For all samples, ESR spectra showed to be composed of three different signals following the Curie's law. One signal was attributed to high-spin ferric ions (g∼ 4.3) in rhomboedric symmetry, Cu(II) ions (close to g=2.0) and neuromelanin (g∼ 2.01). The ferric ions concentration ratio between patients and controls was 3.0±0.2. The same ratio for neuromelanine was 0.24±0.06. Our preliminary results indicated a significant increment of iron concentration in PD samples which agrees with previous histochemical and biochemical reports. This finding and the clear reduction of neuromelanin concentration in PD samples suggest the possible role of neuromelanin as iron ions storage. © 2012 American Association of Physicists in Medicine.

Skyrme forces and decay of the Rf266*104 nucleus synthesized via different incoming channels

NASA Astrophysics Data System (ADS)

Niyti, Deep, Aman; Kharab, Rajesh; Chopra, Sahila; Gupta, Raj K.

2017-03-01

The excitation functions for the production of 262Rf, 261Rf, and 260Rf isotopes via 4 n -, 5 n -, and 6 n -decay channels from the *266Rf compound nucleus are studied within the dynamical cluster-decay model (DCM), including deformations β2 i and so-called hot-optimum orientations θi which support symmetric fission, in agreement with experiments. The data are available for 18O+248Cm and 22Ne+244Pu reactions, respectively, at the energy ranges of Elab=88.2 to 101.3 and 109.0 to 124.8 MeV. For the nuclear interaction potentials, we use the Skyrme energy density functional (SEDF) based on semiclassical extended Thomas Fermi (ETF) approach, which means an extension of the earlier study of excitation functions of *266Rf formed in 18O+248Cm reaction, based on the DCM using the pocket formula for nuclear proximity potential, showing interaction dependence. The Skyrme forces used here are the old SIII and SIV and new GSkI and KDE0(v1) given for both normal and isospin-rich nuclei, with densities added in frozen density approximation. Interestingly, the DCM gives an excellent fit to the measured data on fusion evaporation residue (ER) for both the incoming channels (18O+248Cm and 22Ne+244Pu ) at the energy range Elab=88.2 to 124.8 MeV, independent of the entrance channel and Skyrme force used. The possible fusion-fission (ff) and quasifission (qf) mass regions of fragments on DCM are also predicted. The DCM with Skyrme forces is further used to look for all the possible target-projectile (t-p) combinations forming the cold compound nucleus (CN) *266Rf at the CN excitation energy of Elab for hot compact configurations. The fusion evaporation residue cross sections, for the proposed new reactions in synthesizing the CN *266Rf, are also estimated for the future experiments, and role of mass asymmetry of nuclei is indicated.

Isomer spectroscopy of neutron-rich 168Tb 103

DOE PAGES

Gurgi, L. A.; Regan, P. H.; Söderström, P. -A.; ...

2016-12-29

In-flight fission of a 345 MeV per nucleon 238U primary beam on a 2 mm thick 9Be target has been used to produce and study the decays of a range of neutron-rich nuclei centred around the doubly mid-shell nucleus 170Dy at the RIBF Facility, RIKEN, Japan. The produced secondary fragments of interest were identified event-by-event using the BigRIPS separator. The fragments were implanted into the WAS3ABI position sensitive silicon active stopper which allowed pixelated correlations between implants and their subsequent β-decay. Discrete γ-ray transitions emitted following decays from either metastable states or excited states populated following beta decay were identifiedmore » using the 84 coaxial high-purity germanium (HPGe) detectors of the EURICA spectrometer, which was complemented by 18 additional cerium-doped lanthanum bromide (LaBr 3) fast-timing scintillation detectors from the FATIMA collaboration. This paper presents the internal decay of a metastable isomeric excited state in the odd-odd nucleus 168Tb, which corresponds to a single proton-neutron hole configuration in the valence maximum nucleus 170Dy. These data represent the first information on excited states in this nucleus, which is the most neutron-rich odd-odd isotope of terbium (Z = 65) studied to date. Here, Nilsson configurations associated with an axially symmetric, prolate-deformed nucleus are proposed for the 168Tb ground state the observed isomeric state by comparison with Blocked BCS-Nilsson calculations.« less

Isomer spectroscopy of neutron-rich 168Tb103

NASA Astrophysics Data System (ADS)

Gurgi, L. A.; Regan, P. H.; Söderström, P.-A.; Watanabe, H.; Walker, P. M.; Podolyák, Zs.; Nishimura, S.; Berry, T. A.; Doornenbal, P.; Lorusso, G.; Isobe, T.; Baba, H.; Xu, Z. Y.; Sakurai, H.; Sumikama, T.; Catford, W. N.; Bruce, A. M.; Browne, F.; Lane, G. J.; Kondev, F. G.; Odahara, A.; Wu, J.; Liu, H. L.; Xu, F. R.; Korkulu, Z.; Lee, P.; Liu, J. J.; Phong, V. H.; Yag, A.; Zhang, G. X.; Alharbi, T.; Carroll, R. J.; Chae, K. Y.; Dombradi, Zs.; Estrade, A.; Fukuda, N.; Griffin, C.; Ideguchi, E.; Inabe, N.; Kanaoka, H.; Kojouharov, I.; Kubo, T.; Kubono, S.; Kurz, N.; Kuti, I.; Lalkovski, S.; Lee, E. J.; Lee, C. S.; Lotay, G.; Moon, C.-B.; Nishizuka, I.; Nita, C. R.; Patel, Z.; Roberts, O. J.; Schaffner, H.; Shand, C. M.; Suzuki, H.; Takeda, H.; Terashima, S.; Vajta, Zs.; Yoshida, S.; Valiente-Dòbon, J. J.

2017-11-01

In-flight fission of a 345 MeV per nucleon 238U primary beam on a 2 mm thick 9Be target has been used to produce and study the decays of a range of neutron-rich nuclei centred around the doubly mid-shell nucleus 170Dy at the RIBF Facility, RIKEN, Japan. The produced secondary fragments of interest were identified event-by-event using the BigRIPS separator. The fragments were implanted into the WAS3ABI position sensitive silicon active stopper which allowed pixelated correlations between implants and their subsequent β-decay. Discrete γ-ray transitions emitted following decays from either metastable states or excited states populated following beta decay were identified using the 84 coaxial high-purity germanium (HPGe) detectors of the EURICA spectrometer, which was complemented by 18 additional cerium-doped lanthanum bromide (LaBr3) fast-timing scintillation detectors from the FATIMA collaboration. This paper presents the internal decay of a metastable isomeric excited state in the odd-odd nucleus 168Tb, which corresponds to a single proton-neutron hole configuration in the valence maximum nucleus 170Dy. These data represent the first information on excited states in this nucleus, which is the most neutron-rich odd-odd isotope of terbium (Z=65) studied to date. Nilsson configurations associated with an axially symmetric, prolate-deformed nucleus are proposed for the 168Tb ground state the observed isomeric state by comparison with Blocked BCS-Nilsson calculations.

Investigation of negative-parity states in Dy 156 : Search for evidence of tetrahedral symmetry

DOE PAGES

Hartley, D. J.; Riedinger, L. L.; Janssens, R. V. F.; ...

2017-01-01

An experiment populating low/medium-spin states in 156Dy was performed to investigate the possibility of tetrahedral symmetry in this nucleus. In particular, focus was placed on the low-spin, negative-parity states since recent theoretical studies suggest that these may be good candidates for this high-rank symmetry. The states were produced in the 148Nd( 12C,4 n) reaction and the Gammasphere array was utilized to detect the emitted rays. B(E 2) /B(E1) ratios of transition probabilities from the low-spin, negative-parity bands were determined and used to interpret whether these structures are best associated with tetrahedral symmetry or, as previously assigned, to octupole vibrations. Additionally,more » several other negative-parity structures were observed to higher spin and two new sequences were established« less

Ferromagnetic insulating state in tensile-strained LaCoO3 thin films from LDA + U calculations

NASA Astrophysics Data System (ADS)

Hsu, Han; Blaha, Peter; Wentzcovitch, Renata M.

2012-04-01

With local density approximation+Hubbard U (LDA+U) calculations, we show that the ferromagnetic (FM) insulating state observed in tensile-strained LaCoO3 epitaxial thin films is most likely a mixture of low-spin (LS) and high-spin (HS) Co, namely, a HS/LS mixture state. Compared with other FM states, including the intermediate-spin (IS) state (metallic within LDA+U), which consists of IS Co only, and the insulating IS/LS mixture state, the HS/LS state is the most favorable one. The FM order in the HS/LS state is stabilized via the superexchange interactions between adjacent LS and HS Co. We also show that the Co spin state can be identified by measuring the electric field gradient at the Co nucleus via nuclear magnetic resonance spectroscopy.

Investigation of negative-parity states in Dy 156 : Search for evidence of tetrahedral symmetry

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hartley, D. J.; Riedinger, L. L.; Janssens, R. V. F.

2017-01-01

An experiment populating low/medium-spin states in 156 Dy was performed to investigate the possibility of tetrahedral symmetry in this nucleus. In particular, focus was placed on the low-spin, negative-parity states since recent theoretical studies suggest that these may be good candidates for this high-rank symmetry. The states were produced in the 148 Nd ( 12 C , 4 n ) reaction and the Gammasphere array was utilized to detect the emitted γ rays. B ( E 2 ) / B ( E 1 ) ratios of transition probabilities from the low-spin, negative-parity bands were determined and used to interpret whethermore » these structures are best associated with tetrahedral symmetry or, as previously assigned, to octupole vibrations. In addition, several other negative-parity structures were observed to higher spin and two new sequences were established.« less

Prompt photon measurements with the PHENIX MPC-EX detector

NASA Astrophysics Data System (ADS)

Campbell, Sarah

2013-04-01

The MPC-EX detector is a preshower extension to PHENIX's Muon Piston Calorimeter (MPC). It consists of eight layers of alternating W absorber and Si mini-pad sensors. Located at forward rapidity, 3.1<|η|<3.8, the MPC and MPC-EX access low-x partons in the Au nucleus in p+Au collisions and high-x partons in the projectile in polarized p+p collisions. With the MPC-EX, photon and ^0 separation extends to E>80 GeV, allowing the measurement of prompt photons using the double ratio method. At forward rapidities, prompt photons are dominated by direct photons produced by quark-gluon Compton scattering. In transversely polarized p+p collisions, the prompt photon single spin asymmetry measurement, AN, will resolve the sign discrepancy between the Sivers and twist-3 extractions of AN. In p+Au collisions, the prompt photon RpAu will quantify the level of gluon saturation in the Au nucleus at low-x, 10-3, with a projected systematic error band a factor of four smaller than EPS09's current allowable range. The MPC-EX detector will expand our understanding of gluon nuclear parton distribution functions, providing information about the initial state of heavy ion collisions, and clarify how valence parton's pT and spin correlate to the proton spin.

Lamb shift and fine structure at n =2 in a hydrogenlike muonic atom with the nuclear spin I =0

NASA Astrophysics Data System (ADS)

Korzinin, Evgeny Yu.; Shelyuto, Valery A.; Ivanov, Vladimir G.; Karshenboim, Savely G.

2018-01-01

The paper is devoted to the Lamb shift and fine structure in a hydrogenlike muonic atom with a spinless nucleus up to the order α5m with all the recoil corrections included. Enhanced contributions of a higher order are also considered. We present the results on the pure QED contribution and on the finite-nuclear-size contribution, proportional to RN2, with the higher-order corrections included. We also consider the consistency of the pure QED theory and the evaluation of the nuclear-structure effects. Most of the QED theory is the same as the theory for the case of the nuclear spin 1/2. Additional nuclear-spin-dependent terms are considered in detail. The issue of the difference for the theories with a spinor nucleus and a scalar one is discussed for the recoil contributions in the order (Zα ) 4m ,α (Zα ) 4m , and (Zα ) 5m . The numerical results are presented for the muonic atoms with two lightest scalar nuclei, helium-4 and beryllium-10. We compare the theory of those muonic atoms with theory for the muonic hydrogen. Some higher-order finite-nuclear-size corrections for the Lamb shift in muonic hydrogen are revisited.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Watanabe, H.; Zhang, G. X.; Yoshida, K.

The level structure of 172Dy has been investigated for the first time by means of decay spectroscopy following in-flight fission of a 238U beam. A long-lived isomeric state with T1/2 = 0.71(5) s and Kπ = 8- has been identified at 1278 keV, which decays to the ground-state and γ -vibrational bands through hindered electromagnetic transitions, as well as to the daughter nucleus 172Ho via allowed β decays. The robust nature of the Kπ = 8- isomer and the ground-state rotational band reveals an axially-symmetric structure for this nucleus. Meanwhile, the γ -vibrational levels have been identified at unusually lowmore » excitation energy compared to the neighboring well-deformed nuclei, indicating the significance of the microscopic effect on the non-axial collectivity in this doubly mid-shell region. The underlying mechanism of enhanced γ vibration is discussed in comparison with the deformed Quasiparticle Random-Phase Approximation based on a Skyrme energy-density functional.« less

Possible interpretation of the precession of comet 67P/Churyumov-Gerasimenko

NASA Astrophysics Data System (ADS)

Gutiérrez, P. J.; Jorda, L.; Gaskell, R. W.; Davidsson, B. J. R.; Capanna, C.; Hviid, S. F.; Keller, H. U.; Maquet, L.; Mottola, S.; Preusker, F.; Scholten, F.; Lara, L. M.; Moreno, F.; Rodrigo, R.; Sierks, H.; Barbieri, C.; Lamy, P.; Koschny, D.; Rickman, H.; Agarwal, J.; A'Hearn, M. F.; Auger, A. T.; Barucci, M. A.; Bertaux, J. L.; Bertini, I.; Cremonese, G.; Da Deppo, V.; Debei, S.; De Cecco, M.; El-Maarry, M. R.; Fornasier, S.; Fulle, M.; Groussin, O.; Gutiérrez-Marques, P.; Güttler, C.; Ip, W. H.; Knollenberg, J.; Kramm, J. R.; Kührt, E.; Küppers, M.; La Forgia, F.; Lazzarin, M.; López-Moreno, J. J.; Magrin, S.; Marchi, S.; Marzari, F.; Naletto, G.; Oklay, N.; Pajola, M.; Pommerol, A.; Sabau, D.; Thomas, N.; Toth, I.; Tubiana, C.; Vincent, J. B.

2016-05-01

Context. Data derived from the reconstruction of the nucleus shape of comet 67P/Churyumov-Gerasimenko (67P) from images of the OSIRIS camera onboard ROSETTA show evidence that the nucleus rotates in complex mode. First, the orientation of the spin axis is not fixed in an inertial reference frame, which suggests a precessing motion around the angular momentum vector with a periodicity of approximately 257 h ± 12 h.Second, periodograms of the right ascension and declination (RA/Dec) coordinates of the body-frame Z axis show a very significant (higher than 99.99%) periodicity at 276 h ± 12 h, different from the rotational period of 12.40 h as previously determined from light-curve analysis. Aims: The main goal is to interpret the data and associated periodicities of the spin axis orientation in space. Methods: We analyzed the spin axis orientation in space and associated periodicities and compared them with solutions of Euler equations under the assumption that the body rotates in torque-free conditions. Statistical tests comparing the observationally derived spin axis orientation with the outcome from simulations were applied to determine the most likely inertia moments, excitation level, and periods. Results: Under the assumption that the body is solid-rigid and rotates in torque-free conditions, the most likely interpretation is that 67P is spinning around the principal axis with the highest inertia moment with a period of about 13 h. At the same time, the comet precesses around the angular momentum vector with a period of about 6.35 h. While the rotating period of such a body would be about 12.4 h, RA/Dec coordinates of the spin axis would have a periodicity of about 270 h as a result of the combination of the two aforementioned motions. Conclusions: The most direct and simple interpretation of the complex rotation of 67P requires a ratio of inertia moments significantly higher than that of a homogeneous body.

Study of near-stability nuclei populated as fission fragments in heavy-ion fusion reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fotiadis, Nikolaos; Nelson, Ronald O; Devlin, Matthew

2010-01-01

Examples are presented to illustrate the power of prompt {gamma}-ray spectroscopy of fission fragments from compound nuclei with A {approx} 200 formed in fusion-evaporation reactions in experiments using the Gammasphere Ge-detector array. Complementary methods, such as Coulomb excitation and deep-inelastic processes, are also discussed. In other cases (n, xn{gamma}) reactions on stable isotopes have been used to establish neutron excitation functions for {gamma}-rays using a pulsed 'white'-neutron source, coupled to a high-energy-resolution germanium-detector array. The excitation functions can unambiguously assign {gamma}-rays to a specific reaction product. Results from all these methods bridge the gaps in the systematics of high-spin statesmore » between the neutron-deficient and neutron-rich nuclei. Results near shell closures should motivate new shell model calculations.« less

Thermal transport in UO 2 with defects and fission products by molecular dynamics simulations

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Xiang-Yang; Cooper, Michael William Donald; Mcclellan, Kenneth James

2015-10-14

The importance of the thermal transport in nuclear fuel has motivated a wide range of experimental and modelling studies. In this report, the reduction of thermal transport in UO 2 due to defects and fission products has been investigated using non-equilibrium MD simulations, with two sets of empirical potentials for studying the degregation of UO 2 thermal conductivity including a Buckingham type interatomic potential and a recently developed EAM type interatomic potential. Additional parameters for U 5+ and Zr 4+ in UO 2 have been developed for the EAM potential. The thermal conductivity results from MD simulations are then correctedmore » for the spin-phonon scattering through Callaway model formulations. To validate the modelling results, comparison was made with experimental measurements on single crystal hyper-stoichiometric UO 2+x samples.« less

High-spin studies: Recent results from the 8π spectrometer

NASA Astrophysics Data System (ADS)

Radford, D. C.; Galindo-Uribarri, A.; Hackman, G.; Janzen, V. P.; 8π Collaboration

1993-05-01

Selected highlights of recent high-spin nuclear-structure studies with the 8π spectrometer are presented. These include an extensive systematic study of high- j intruder bands in A ˜ 110 Sb, Sn and In nuclei; evidence for hyperdeformation, observed in the reaction 120Sn( 37Cl,px n) populating 152,153Dy; and the observation of a new superdeformed band in the N = 80 nucleus 142Sm. The design of "TRIGAM", a new HPGe-detector array proposed to replace the 8π spectrometer, is also presented.

Cement As a Waste Form for Nuclear Fission Products: The Case of (90)Sr and Its Daughters.

PubMed

Dezerald, Lucile; Kohanoff, Jorge J; Correa, Alfredo A; Caro, Alfredo; Pellenq, Roland J-M; Ulm, Franz J; Saúl, Andrés

2015-11-17

One of the main challenges faced by the nuclear industry is the long-term confinement of nuclear waste. Because it is inexpensive and easy to manufacture, cement is the material of choice to store large volumes of radioactive materials, in particular the low-level medium-lived fission products. It is therefore of utmost importance to assess the chemical and structural stability of cement containing radioactive species. Here, we use ab initio calculations based on density functional theory (DFT) to study the effects of (90)Sr insertion and decay in C-S-H (calcium-silicate-hydrate) in order to test the ability of cement to trap and hold this radioactive fission product and to investigate the consequences of its β-decay on the cement paste structure. We show that (90)Sr is stable when it substitutes the Ca(2+) ions in C-S-H, and so is its daughter nucleus (90)Y after β-decay. Interestingly, (90)Zr, daughter of (90)Y and final product in the decay sequence, is found to be unstable compared to the bulk phase of the element at zero K but stable when compared to the solvated ion in water. Therefore, cement appears as a suitable waste form for (90)Sr storage.

Rapid evolution of the spin state of comet 41P/Tuttle-Giacobini-Kresak

NASA Astrophysics Data System (ADS)

Bodewits, Dennis; Farnham, Tony; Knight, Matthew M.; Kelley, Michael S.

2017-10-01

Comet nuclei are small, dynamic objects influenced strongly by their individual history, orbit, rotation and inhomogeneity. Mass loss due to sublimation can exert a profound influence on the physical nature of the cometary nucleus, changing the shape, size, and rotation (Jewitt, in Comets II, 2004). The Rosetta mission to comet 67P showed that these effects are all interrelated (Sierks et al., Science 347, 2015).Comet 41P/Tuttle-Giacobini-Kresak passed Earth as close as 0.142 au in April 2017, allowing observations of the inner coma and an assessment of the rotational state of the nucleus. We acquired observations of comet 41P between March and May 2017 using the 4.3-m Discovery Channel Telescope and the UltraViolet-Optical Telescope (UVOT) on board the Earth-orbiting Swift Gamma Ray Burst Mission.Using CN narrowband imaging and aperture photometry we found that the apparent rotation period of comet 41P more than doubled between March and May 2017, increasing from 20 hours to 50 hours. Measurements of the periodicity in late-March by Knight et al. (CBET 4377, 2017) are consistent with this rate of increase. Comet 41P is the ninth comet for which a rotation period change has been observed (c.f. Samarasinha et al., in Comets II, 2004), but both the fractional change and the rate of change of the period far exceed those observed in the other comets. It is presumably the combination of a long rotation period, high surface activity, and a small nucleus that makes 41P highly susceptible to changes in its rotational state.Extrapolating the comet’s rotation period using its current gas production rates and a simple activity model suggests that the nucleus will continue to spin down, possibly leading to an excited spin state in the next few apparitions. Finally, 41P is known for its large outbursts, and our extrapolation suggest that the comet’s rotation period may have been close to the critical period for splitting in 2001, when it exhibited two significant outbursts.

Excitations of one-valence-proton, one-valence-neutron nucleus {sup 210}Bi from cold-neutron capture

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cieplicka-Oryńczak, N.; Institute of Nuclear Physics, Polish Academy of Sciences, PL-31342 Kraków; Fornal, B.

2015-10-15

The low-spin structure of one-proton, one-neutron {sup 210}Bi nucleus was investigated in cold-neutron capture reaction on {sup 209}Bi. The γ-coincidence measurements were performed with use of EXILL array consisted of 16 HPGe detectors. The experimental results were compared to shell-model calculations involving valence particles excitations. The {sup 210}Bi nucleus offers the potential to test the effective proton-neutron interactions because most of the states should arise from the proton-neutron excitations. Additionally, it was discovered that a few states should come from the couplings of valence particles to the 3{sup −} octupole vibration in {sup 208}Pb which provides also the possibility ofmore » testing the calculations involving the core excitations.« less

Identification of Excited States in the N=Z Nucleus 82Nb

NASA Astrophysics Data System (ADS)

Caceres, L. S.; Gorska, M.; Jungclaus, A.; Regan, P. H.; Garnsworthy, A. B.; Pietri, S.; Podolyak, Zs.; Rudolph, D.; Steer, S. J.; Grawe, H.; Balabanski, D. L.; Becker, F.; Bednarczyk, P.; Benzoni, G.; Blank, B.; Brandau, C.; Bruce, A. M.; Camera, F.; Catford, W. N.; Cullen, I. J.; Dombradi, Zs.; Doornenbal, P.; Estevez, E.; Geissel, H.; Gelletly, W.; Gerl, J.; Grebosz, J.; Heinz, A.; Hoischen, R.; Ilie, G.; Jolie, J.; Jones, G. A.; Kmiecik, M.; Kojouharov, I.; Kondev, F. G.; Kurtukian-Nieto, T.; Kurz, N.; Lalkowski, S.; Liu, L.; Maj, A.; Myalski, S.; Montes, F.; Pfuetzner, M.; Prokopowicz, W.; Saito, T.; Schaffner, H.; Schwertel, S.; Shizuma, T.; Simons, A. J.; Tashenov, S.; Walker, P. M.; Werner-Malento, E.; Wieland, O.; Wollersheim, H. J.

2007-04-01

Information on the first excited states in the N=Z=41 nucleus 82Nb sheds light on the competition of isospin T=0 and T=1 states in the A sim 80 region. The measurement was performed at the GSI laboratory using fragmentation of a 107Ag primary beam at 750 MeV/u on a 4 g/cm2 9Be target. The fragments were separated and identified unambiguously in the FRagment Separator. Three excited states were observed and the half-life estimate for the isomeric state was extracted. A tentative spin assignment based on the isobaric analogue states systematics in the Tz=1 nucleus 82Zr, and transition probabilities indicate T=1 character of the first two excited states, and T=0 for the isomeric state.

Reflection Asymmetric Shapes in the Neutron-Rich 140,143Ba Isotopes

NASA Astrophysics Data System (ADS)

Zhu Sheng-jiang (S, J. Zhu; Wang, Mu-ge; J, H. Hamilton; A, V. Ramayya; B, R. S. Babu; W, C. Ma; Long, Gui-lu; Deng, Jing-kang; Zhu, Ling-yan; Li, Ming; T, N. Ginter; J, Komicki; J, D. Cole; R, Aryaeinejad; Y, K. Dardenne; M, W. Drigert; J, O. Rasmussen; Ts, Yu Oganessian; M, A. Stoyer; S, Y. Chu; K, E. Gregorich; M, F. Mohar; S, G. Prussin; I, Y. Lee; N, R. Johnson; F, K. McGowan

1997-08-01

Level schemes for the neutron-rich 140,143Ba nuclei have been determined by study of prompt γ-rays in spontaneous fission of 252Cf. The level pattern and enhanced E1 transitions between π = + and π = - bands show reflection asymmetric shapes with simplex quantum number s = +1 in 140Ba and s = ±i in 143Ba, respectively. The octupole deformation stability with spin variation has been discussed.

Analysis of the experimental level scheme of {sup 61}Cu using computational technique

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gupta, Anuradha, E-mail: annu1gupta1@gmail.com; Verma, Preeti, E-mail: preetiverma130587@gmail.com; Bharti, Arun, E-mail: arunbharti-2003@yahoo.co.in

2015-08-28

The high-spin structure in {sup 61}Cu nucleus is studied in terms of effective two body interaction. In order to take into account the deformed BCS basis, the basis states are expanded in terms of the core eigenfunctions. Yrast band with some other bands havew been obtained and back-bending in moment of inertia has also been calculated and compared with the available experimental data for {sup 61}Cu nucleus. On comparing the available experimental as well as other theoretical data, it is found that the treatment with PSM provides a satisfactory explanation of the available data.

Nuclear physics with antiprotons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dover, C.B.

1984-01-01

Transparencies of an invited talk presented at the Nashville meeting of the American Physical Society, October 18-20, 1984, are included. Topics include: (1) Salient features of two-body N anti N interactions (N anti N reversible NN, annihilation mechanisms (quark models), and optical model phenomenology); (2) anti N-nucleus interactions - elastic, inelastic, etc. (new cross section data, optical potentials, signatures of spin-isospin dependence of N anti N force, and (anti p, p) reactions); and (3) anti N-nucleus annihilation processes (features of cascade or fluid dynamics calculations, searches for baryonium and other exotics, meson interferometry, and (anti p, NN) reactions. (WHK)

Spin-isospin excitation of 3He with three-proton final state

NASA Astrophysics Data System (ADS)

Ishikawa, Souichi

2018-01-01

Spin-isospin excitation of the {}^3He nucleus by a proton-induced charge exchange reaction, {}^3He(p,n)ppp, at forward neutron scattering angle is studied in a plane wave impulse approximation (PWIA). In PWIA, cross sections of the reaction are written in terms of proton-neutron scattering amplitudes and response functions of the transition from {}3He to the three-proton state by spin-isospin transition operators. The response functions are calculated with realistic nucleon-nucleon potential models using a Faddeev three-body method. Calculated cross sections agree with available experimental data in substance. Possible effects arising from the uncertainty of proton-neutron amplitudes and three-nucleon interactions in the three-proton system are examined.

Study of the Spin Dependent 3HE-NUCLEUS Interaction at 450 Mev

NASA Astrophysics Data System (ADS)

Kamiya, J.; Hatanaka, K.; Sakemi, Y.; Wakasa, T.; Yoshida, H. P.; Obayashi, E.; Hara, K.; Kitamura, K.; Shimizu, Y.; Fujita, K.; Sakamoto, N.; Shimbara, Y.; Adachi, T.; Sakaguchi, H.; Yosoi, M.; Uchida, M.; Yasuda, Y.; Kawabata, T.; Noro, T.

2003-04-01

Differential cross sections and induced polarizations of 3He+12C, 58Ni, and 90Zr elastic scattering were measured at E3He = 450 MeV. This is the first measurement of the polarization for 3He scattering at intermediate energies. The optical potential parameters including the spin-orbit potential were determined with small uncertainties. The volume integrals per nucleon of the potentials were investigated for 3He and their energy dependence showed the similar behavior to that for protons at intermediate energies. The single folding calculations were compared with the data. The real central and spin-orbit parts of the folded potentials had to be reduced by a few tens of percent in order to reproduce the experimental results.

Using polarized muons as ultrasensitive spin labels in free radical chemistry

NASA Astrophysics Data System (ADS)

McKenzie, Iain; Roduner, Emil

2009-08-01

In a chemical sense, the positive muon is a light proton. It is obtained at the ports of accelerators in beams with a spin polarization of 100%, which makes it a highly sensitive probe of matter. The muonium atom is a light hydrogen isotope, nine times lighter than H, with a muon as its nucleus. It reacts the same way as H, and by addition to double bonds it is implemented in free radicals in which the muon serves as a fully polarized spin label. It is reviewed here how the muon can be used to obtain information about muonium and radical reaction rates, radical structure, dynamics, and local environments. It can even tell us what a fragrance molecule does in a shampoo.

Triaxiality and Exotic Rotations at High Spins in 134Ce

DOE PAGES

Petrache, C. M.; Guo, S.; Ayangeakaa, A. D.; ...

2016-06-06

High-spin states in Ce-134 have been investigated using the Cd-116(Ne-22,4n) reaction and the Gammasphere array. The level scheme has been extended to an excitation energy of similar to 30 MeV and spin similar to 54 (h) over bar. Two new dipole bands and four new sequences of quadrupole transitions were identified. Several new transitions have been added to a number of known bands. One of the strongly populated dipole bands was revised and placed differently in the level scheme, resolving a discrepancy between experiment and model calculations reported previously. Configurations are assigned to the observed bands based on cranked Nilsson-Strutinskymore » calculations. A coherent understanding of the various excitations, both at low and high spins, is thus obtained, supporting an interpretation in terms of coexistence of stable triaxial, highly deformed, and superdeformed shapes up to very high spins. Rotations around different axes of the triaxial nucleus, and sudden changes of the rotation axis in specific configurations, are identified, further elucidating the nature of high-spin collective excitations in the A = 130 mass region.« less

Investigation of high spin states in 133Cs

NASA Astrophysics Data System (ADS)

Xu, Q.; Xiao, Z. G.; Zhu, S. J.; Qi, C.; Jia, H.; Qi, B.; Wang, R. S.; Cheng, W. J.; Zhang, Y.; Yi, H.; Lü, L. M.; Wang, Y. J.; Li, H. J.; Huang, Y.; Zhang, Z.; Wu, X. G.; Li, C. B.; Zheng, Y.; Chen, Q. M.; Zhou, W. K.; Li, G. S.

2018-05-01

High spin states in 133Cs nucleus have been studied with the reaction 130Te (7Li, 4n) at a beam energy of 38 MeV. The level scheme has been expanded with spin up to 31/2 \\hbar. Compared with a recent paper, ground state band and other two collective band structures at lower spin states have been confirmed. Another collective band structure at higher spin states as well as some levels and transitions are updated. Compared with the experimental data, large-scale shell model and tilted axis cranking model calculations have been carried out. The results show that the band-head configuration of yrast band based on 7/2+ ground state and the side band built on the 5/2+ state are a pair of pseudospin partner states with π \\tilde{f}_{7/2,5/2}. The negative parity band based on 1071.5 keV level originates from π h_{11/2} orbital. Another band built on 2642.9 keV level at high spin states has been proposed with oblate deformation. Other characteristics for these bands were also discussed.

Polarization singularities and orbital angular momentum sidebands from rotational symmetry broken by the Pockels effect

PubMed Central

Lu, Xiancong; Wu, Ziwen; Zhang, Wuhong; Chen, Lixiang

2014-01-01

The law of angular momentum conservation is naturally linked to the rotational symmetry of the involved system. Here we demonstrate theoretically how to break the rotational symmetry of a uniaxial crystal via the electro-optic Pockels effect. By numerical method based on asymptotic expansion, we discover the 3D structure of polarization singularities in terms of C lines and L surfaces embedded in the emerging light. We visualize the controllable dynamics evolution of polarization singularities when undergoing the Pockels effect, which behaves just like the binary fission of a prokaryotic cell, i.e., the splitting of C points and fission of L lines are animated in analogy with the cleavage of nucleus and division of cytoplasm. We reveal the connection of polarization singularity dynamics with the accompanying generation of orbital angular momentum sidebands. It is unexpected that although the total angular momentum of light is not conserved, the total topological index of C points is conserved. PMID:24784778

Polarization singularities and orbital angular momentum sidebands from rotational symmetry broken by the Pockels effect.

PubMed

Lu, Xiancong; Wu, Ziwen; Zhang, Wuhong; Chen, Lixiang

2014-05-02

The law of angular momentum conservation is naturally linked to the rotational symmetry of the involved system. Here we demonstrate theoretically how to break the rotational symmetry of a uniaxial crystal via the electro-optic Pockels effect. By numerical method based on asymptotic expansion, we discover the 3D structure of polarization singularities in terms of C lines and L surfaces embedded in the emerging light. We visualize the controllable dynamics evolution of polarization singularities when undergoing the Pockels effect, which behaves just like the binary fission of a prokaryotic cell, i.e., the splitting of C points and fission of L lines are animated in analogy with the cleavage of nucleus and division of cytoplasm. We reveal the connection of polarization singularity dynamics with the accompanying generation of orbital angular momentum sidebands. It is unexpected that although the total angular momentum of light is not conserved, the total topological index of C points is conserved.

Revival of Dobell's "chromidia" hypothesis: chromatin bodies in the amoebomastigote Paratetramitus jugosus

NASA Technical Reports Server (NTRS)

Margulis, L.; Enzien, M.; McKhann, H. I.

1990-01-01

Multiple fission of a mature Paratetramitus jugosus (approx. 10 micrometers long) resulted in the production of many small, roughly spherical (2-7 micrometers in diameter) amoebae. Our observation of live material and examination of over two hundred micrographs lead us to suggest that DNA-containing membrane-bounded chromatin bodies bud amitotically from the nucleus. DAPI-stained bodies of these were observed in the cytoplasm of amoebae, mastigotes, and cysts, and at least some of these chromatin bodies seemed to be released into the medium. This interpretation revives for P. jugosus the "chromatin hypothesis" of Dobell. Our data, consistent with the descriptions of Dobell, Hogue, and Wherry, indicate that encysting amoebae may reproduce by chromidia. Dobell's original chromidia concept was limited to amoebae. Others claimed for it far-reaching consequences: "chromidia" were touted as an explanation for embryogenesis and histogenesis of metazoa. Although there is no evidence for chromidia in animals, outright rejection of Dobell's chromidia hypothesis sensu stricto as an amitotic multiple fission process in amoebae is unjustified.

Polarization singularities and orbital angular momentum sidebands from rotational symmetry broken by the Pockels effect

NASA Astrophysics Data System (ADS)

Lu, Xiancong; Wu, Ziwen; Zhang, Wuhong; Chen, Lixiang

2014-05-01

The law of angular momentum conservation is naturally linked to the rotational symmetry of the involved system. Here we demonstrate theoretically how to break the rotational symmetry of a uniaxial crystal via the electro-optic Pockels effect. By numerical method based on asymptotic expansion, we discover the 3D structure of polarization singularities in terms of C lines and L surfaces embedded in the emerging light. We visualize the controllable dynamics evolution of polarization singularities when undergoing the Pockels effect, which behaves just like the binary fission of a prokaryotic cell, i.e., the splitting of C points and fission of L lines are animated in analogy with the cleavage of nucleus and division of cytoplasm. We reveal the connection of polarization singularity dynamics with the accompanying generation of orbital angular momentum sidebands. It is unexpected that although the total angular momentum of light is not conserved, the total topological index of C points is conserved.

Theory for cross effect dynamic nuclear polarization under magic-angle spinning in solid state nuclear magnetic resonance: the importance of level crossings.

PubMed

Thurber, Kent R; Tycko, Robert

2012-08-28

We present theoretical calculations of dynamic nuclear polarization (DNP) due to the cross effect in nuclear magnetic resonance under magic-angle spinning (MAS). Using a three-spin model (two electrons and one nucleus), cross effect DNP with MAS for electron spins with a large g-anisotropy can be seen as a series of spin transitions at avoided crossings of the energy levels, with varying degrees of adiabaticity. If the electron spin-lattice relaxation time T(1e) is large relative to the MAS rotation period, the cross effect can happen as two separate events: (i) partial saturation of one electron spin by the applied microwaves as one electron spin resonance (ESR) frequency crosses the microwave frequency and (ii) flip of all three spins, when the difference of the two ESR frequencies crosses the nuclear frequency, which transfers polarization to the nuclear spin if the two electron spins have different polarizations. In addition, adiabatic level crossings at which the two ESR frequencies become equal serve to maintain non-uniform saturation across the ESR line. We present analytical results based on the Landau-Zener theory of adiabatic transitions, as well as numerical quantum mechanical calculations for the evolution of the time-dependent three-spin system. These calculations provide insight into the dependence of cross effect DNP on various experimental parameters, including MAS frequency, microwave field strength, spin relaxation rates, hyperfine and electron-electron dipole coupling strengths, and the nature of the biradical dopants.

A single-atom quantum memory in silicon

DOE Office of Scientific and Technical Information (OSTI.GOV)

Freer, Solomon; Simmons, Stephanie; Laucht, Arne

Long coherence times and fast gate operations are desirable but often conflicting requirements for physical qubits. This conflict can be resolved by resorting to fast qubits for operations, and by storing their state in a ‘quantum memory’ while idle. The 31P donor in silicon comes naturally equipped with a fast qubit (the electron spin) and a long-lived qubit (the 31P nuclear spin), coexisting in a bound state at cryogenic temperatures. Here, we demonstrate storage and retrieval of quantum information from a single donor electron spin to its host phosphorus nucleus in isotopically-enriched 28Si. The fidelity of the memory process ismore » characterised via both state and process tomography. We report an overall process fidelity Fp ! 81%, a memory fidelity Fm ! 92%, and memory storage times up to 80 ms. These values are limited by a transient shift of the electron spin resonance frequency following highpower radiofrequency pulses.« less

A single-atom quantum memory in silicon

DOE PAGES

Freer, Solomon; Simmons, Stephanie; Laucht, Arne; ...

2017-03-20

Long coherence times and fast gate operations are desirable but often conflicting requirements for physical qubits. This conflict can be resolved by resorting to fast qubits for operations, and by storing their state in a ‘quantum memory’ while idle. The 31P donor in silicon comes naturally equipped with a fast qubit (the electron spin) and a long-lived qubit (the 31P nuclear spin), coexisting in a bound state at cryogenic temperatures. Here, we demonstrate storage and retrieval of quantum information from a single donor electron spin to its host phosphorus nucleus in isotopically-enriched 28Si. The fidelity of the memory process ismore » characterised via both state and process tomography. We report an overall process fidelity Fp ! 81%, a memory fidelity Fm ! 92%, and memory storage times up to 80 ms. These values are limited by a transient shift of the electron spin resonance frequency following highpower radiofrequency pulses.« less

Isomer-delayed gamma-ray spectroscopy of neutron-rich 166Tb

DOE PAGES

Gurgi, L. A.; Regan, P. H.; Söderström, P. -A.; ...

2017-09-13

Here, this short paper presents the identification of a metastable, isomeric-state decay in the neutron-rich odd-odd, prolate-deformed nucleus 166Tb. The nucleus of interest was formed using the in-flight fission of a 345 MeV per nucleon 238U primary beam at the RIBF facility, RIKEN, Japan. Gamma-ray transitions decaying from the observed isomeric states in 166Tb were identified using the EURICA gamma-ray spectrometer, positioned at the final focus of the BigRIPS fragments separator. The current work identifies a single discrete gamma-ray transition of energy 119 keV which de-excites an isomeric state in 166Tb with a measured half-life of 3.5(4) μs. The multipolaritymore » assignment for this transition is an electric dipole and is made on the basis internal conversion and decay lifetime arguments. Possible two quasi-particle Nilsson configurations for the initial and final states which are linked by this transition in 166Tb are made on the basis of comparison with Blocked BCS Nilsson calculations, with the predicted ground state configuration for this nucleus arising from the coupling of the v(1-/2)[521] and π(3+/2) Nilsson orbitals.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gurgi, L. A.; Regan, P. H.; Söderström, P. -A.

Here, this short paper presents the identification of a metastable, isomeric-state decay in the neutron-rich odd-odd, prolate-deformed nucleus 166Tb. The nucleus of interest was formed using the in-flight fission of a 345 MeV per nucleon 238U primary beam at the RIBF facility, RIKEN, Japan. Gamma-ray transitions decaying from the observed isomeric states in 166Tb were identified using the EURICA gamma-ray spectrometer, positioned at the final focus of the BigRIPS fragments separator. The current work identifies a single discrete gamma-ray transition of energy 119 keV which de-excites an isomeric state in 166Tb with a measured half-life of 3.5(4) μs. The multipolaritymore » assignment for this transition is an electric dipole and is made on the basis internal conversion and decay lifetime arguments. Possible two quasi-particle Nilsson configurations for the initial and final states which are linked by this transition in 166Tb are made on the basis of comparison with Blocked BCS Nilsson calculations, with the predicted ground state configuration for this nucleus arising from the coupling of the v(1-/2)[521] and π(3+/2) Nilsson orbitals.« less

Isomer-delayed gamma-ray spectroscopy of neutron-rich 166Tb

NASA Astrophysics Data System (ADS)

Gurgi, L. A.; Regan, P. H.; Söderström, P.-A.; Watanabe, H.; Walker, P. M.; Podolyák, Zs.; Nishimura, S.; Berry, T. A.; Doornenbal, P.; Lorusso, G.; Isobe, T.; Baba, H.; Xu, Z. Y.; Sakurai, H.; Sumikama, T.; Catford, W. N.; Bruce, A. M.; Browne, F.; Lane, G. J.; Kondev, F. G.; Odahara, A.; Wu, J.; Liu, H. L.; Xu, F. R.; Korkulu, Z.; Lee, P.; Liu, J. J.; Phong, V. H.; Yagi, A.; Zhang, G. X.; Alharbi, T.; Carroll, R. J.; Chae, K. Y.; Dombradi, Zs.; Estrade, A.; Fukuda, N.; Griffin, C.; Ideguchi, E.; Inabe, N.; Kanaoka, H.; Kojouharov, I.; Kubo, T.; Kubono, S.; Kurz, N.; Kuti, I.; Lalkovski, S.; Lee, E. J.; Lee, C. S.; Lotay, G.; Moon, C. B.; Nishizuka, I.; Nita, C. R.; Patel, Z.; Roberts, O. J.; Schaffner, H.; Shand, C. M.; Suzuki, H.; Takeda, H.; Terashima, S.; Vajta, Zs.; Kanaya, S.; Valiente-Dobòn, J. J.

2017-09-01

This short paper presents the identification of a metastable, isomeric-state decay in the neutron-rich odd-odd, prolate-deformed nucleus 166Tb. The nucleus of interest was formed using the in-flight fission of a 345 MeV per nucleon 238U primary beam at the RIBF facility, RIKEN, Japan. Gamma-ray transitions decaying from the observed isomeric states in 166Tb were identified using the EURICA gamma-ray spectrometer, positioned at the final focus of the BigRIPS fragments separator. The current work identifies a single discrete gamma-ray transition of energy 119 keV which de-excites an isomeric state in 166Tb with a measured half-life of 3.5(4) μs. The multipolarity assignment for this transition is an electric dipole and is made on the basis internal conversion and decay lifetime arguments. Possible two quasi-particle Nilsson configurations for the initial and final states which are linked by this transition in 166Tb are made on the basis of comparison with Blocked BCS Nilsson calculations, with the predicted ground state configuration for this nucleus arising from the coupling of the v(1-/2)?[521] and ? π(3+/2) Nilsson orbitals.

Binary asteroid population. 3. Secondary rotations and elongations

NASA Astrophysics Data System (ADS)

Pravec, P.; Scheirich, P.; Kušnirák, P.; Hornoch, K.; Galád, A.; Naidu, S. P.; Pray, D. P.; Világi, J.; Gajdoš, Š.; Kornoš, L.; Krugly, Yu. N.; Cooney, W. R.; Gross, J.; Terrell, D.; Gaftonyuk, N.; Pollock, J.; Husárik, M.; Chiorny, V.; Stephens, R. D.; Durkee, R.; Reddy, V.; Dyvig, R.; Vraštil, J.; Žižka, J.; Mottola, S.; Hellmich, S.; Oey, J.; Benishek, V.; Kryszczyńska, A.; Higgins, D.; Ries, J.; Marchis, F.; Baek, M.; Macomber, B.; Inasaridze, R.; Kvaratskhelia, O.; Ayvazian, V.; Rumyantsev, V.; Masi, G.; Colas, F.; Lecacheux, J.; Montaigut, R.; Leroy, A.; Brown, P.; Krzeminski, Z.; Molotov, I.; Reichart, D.; Haislip, J.; LaCluyze, A.

2016-03-01

We collected data on rotations and elongations of 46 secondaries of binary and triple systems among near-Earth, Mars-crossing and small main belt asteroids. 24 were found or are strongly suspected to be synchronous (in 1:1 spin-orbit resonance), and the other 22, generally on more distant and/or eccentric orbits, were found or are suggested to have asynchronous rotations. For 18 of the synchronous secondaries, we constrained their librational angles, finding that their long axes pointed to within 20° of the primary on most epochs. The observed anti-correlation of secondary synchroneity with orbital eccentricity and the limited librational angles agree with the theories by Ćuk and Nesvorný (Ćuk, M., Nesvorný, D. [2010]. Icarus 207, 732-743) and Naidu and Margot (Naidu, S.P., Margot, J.-L. [2015]. Astron. J. 149, 80). A reason for the asynchronous secondaries being on wider orbits than synchronous ones may be longer tidal circularization time scales at larger semi-major axes. The asynchronous secondaries show relatively fast spins; their rotation periods are typically < 10 h. An intriguing observation is a paucity of chaotic secondary rotations; with an exception of (35107) 1991 VH, the secondary rotations are single-periodic with no signs of chaotic rotation and their periods are constant on timescales from weeks to years. The secondary equatorial elongations show an upper limit of a2 /b2 ∼ 1.5 . The lack of synchronous secondaries with greater elongations appears consistent, considering uncertainties of the axis ratio estimates, with the theory by Ćuk and Nesvorný that predicts large regions of chaotic rotation in the phase space for a2 /b2 ≳√{ 2 } . Alternatively, secondaries may not form or stay very elongated in gravitational (tidal) field of the primary. It could be due to the secondary fission mechanism suggested by Jacobson and Scheeres (Jacobson, S.A., Scheeres, D.J. [2011]. Icarus 214, 161-178), as its efficiency is correlated with the secondary elongation. Sharma (Sharma, I. [2014]. Icarus 229, 278-294) found that rubble-pile satellites with a2 /b2 ≲ 1.5 are more stable to finite structural perturbations than more elongated ones. It appears that more elongated secondaries, if they originally formed in spin fission of parent asteroid, are less likely to survive intact and they more frequently fail or fission.

Fingerprints of single nuclear spin energy levels using STM - ENDOR

NASA Astrophysics Data System (ADS)

Manassen, Yishay; Averbukh, Michael; Jbara, Moamen; Siebenhofer, Bernhard; Shnirman, Alexander; Horovitz, Baruch

2018-04-01

We performed STM-ENDOR experiments where the intensity of one of the hyperfine components detected in ESR-STM is recorded while an rf power is irradiated into the tunneling junction and its frequency is swept. When the latter frequency is near a nuclear transition a dip in ESR-STM signal is observed. This experiment was performed in three different systems: near surface SiC vacancies where the electron spin is coupled to a next nearest neighbor 29Si nucleus; Cu deposited on Si(111)7x7 surface, where the unpaired electron of the Cu atom is coupled to the Cu nucleus (63Cu, 65Cu) and on Tempo molecules adsorbed on Au(111), where the unpaired electron is coupled to a Nitrogen nucleus (14N). While some of the hyperfine values are unresolved in the ESR-STM data due to linewidth we find that they are accurately determined in the STM-ENDOR data including those from remote nuclei, which are not detected in the ESR-STM spectrum. Furthermore, STM-ENDOR can measure single nuclear Zeeman frequencies, distinguish between isotopes through their different nuclear magnetic moments and detect quadrupole spectra. We also develop and solve a Bloch type equation for the coupled electron-nuclear system that facilitates interpretation of the data. The improved spectral resolution of STM - ENDOR opens many possibilities for nanometric scale chemical analysis.

Fingerprints of single nuclear spin energy levels using STM - ENDOR.

PubMed

Manassen, Yishay; Averbukh, Michael; Jbara, Moamen; Siebenhofer, Bernhard; Shnirman, Alexander; Horovitz, Baruch

2018-04-01

We performed STM-ENDOR experiments where the intensity of one of the hyperfine components detected in ESR-STM is recorded while an rf power is irradiated into the tunneling junction and its frequency is swept. When the latter frequency is near a nuclear transition a dip in ESR-STM signal is observed. This experiment was performed in three different systems: near surface SiC vacancies where the electron spin is coupled to a next nearest neighbor 29 Si nucleus; Cu deposited on Si(111)7x7 surface, where the unpaired electron of the Cu atom is coupled to the Cu nucleus ( 63 Cu, 65 Cu) and on Tempo molecules adsorbed on Au(111), where the unpaired electron is coupled to a Nitrogen nucleus ( 14 N). While some of the hyperfine values are unresolved in the ESR-STM data due to linewidth we find that they are accurately determined in the STM-ENDOR data including those from remote nuclei, which are not detected in the ESR-STM spectrum. Furthermore, STM-ENDOR can measure single nuclear Zeeman frequencies, distinguish between isotopes through their different nuclear magnetic moments and detect quadrupole spectra. We also develop and solve a Bloch type equation for the coupled electron-nuclear system that facilitates interpretation of the data. The improved spectral resolution of STM - ENDOR opens many possibilities for nanometric scale chemical analysis. Copyright © 2018 Elsevier Inc. All rights reserved.

Relativistic Zeroth-Order Regular Approximation Combined with Nonhybrid and Hybrid Density Functional Theory: Performance for NMR Indirect Nuclear Spin-Spin Coupling in Heavy Metal Compounds.

PubMed

Moncho, Salvador; Autschbach, Jochen

2010-01-12

A benchmark study for relativistic density functional calculations of NMR spin-spin coupling constants has been performed. The test set contained 47 complexes with heavy metal atoms (W, Pt, Hg, Tl, Pb) with a total of 88 coupling constants involving one or two heavy metal atoms. One-, two-, three-, and four-bond spin-spin couplings have been computed at different levels of theory (nonhybrid vs hybrid DFT, scalar vs two-component relativistic). The computational model was based on geometries fully optimized at the BP/TZP scalar relativistic zeroth-order regular approximation (ZORA) and the conductor-like screening model (COSMO) to include solvent effects. The NMR computations also employed the continuum solvent model. Computations in the gas phase were performed in order to assess the importance of the solvation model. The relative median deviations between various computational models and experiment were found to range between 13% and 21%, with the highest-level computational model (hybrid density functional computations including scalar plus spin-orbit relativistic effects, the COSMO solvent model, and a Gaussian finite-nucleus model) performing best.

Stability Limits for Rubble Pile Asteroid Shapes

NASA Astrophysics Data System (ADS)

Scheeres, Daniel

2018-04-01

The stability of rubble pile asteroids are explored analytically, using simple models for their constituent components. Specifically, we look at the stability of spherical components resting and potentially rolling on each other as a function of their relative sizes, configuration and number. This talk will present some recent results in this problem. Of specific interest is a 5:1 limit on the elongation of a rubble pile body for stability, which is interestingly the same extreme elongation found for the first interstellar object. This limit is for a rubble pile consisting of stacked spheres, resting on each other in a straight line. If there are 5 or less bodies resting on each other in this configuration, there is an interval of spin rates for which the configuration is stable. If there are 6 or more bodies stacked as such, the spin rate for it to stabilize is beyond the spin rate at which it fissions. The talk will also explore additional results for different configurations of bodies resting on each other.

Properties of Fiber Cell Plasma Membranes Isolated from the Cortex and Nucleus of the Porcine Eye Lens

PubMed Central

Mainali, Laxman; Raguz, Marija; O’Brien, William J.; Subczynski, Witold K.

2012-01-01

The organization and physical properties of the lipid bilayer portion of intact cortical and nuclear fiber cell plasma membranes isolated from the eyes lenses of two-year-old pigs were studied using electron paramagnetic resonance (EPR) spin-labeling. Membrane fluidity, hydrophobicity, and the oxygen transport parameter (OTP) were assessed from the EPR spectra of precisely positioned spin labels. Intact cortical and nuclear membranes, which include membrane proteins, were found to contain three distinct lipid environments. These lipid environments were termed the bulk lipid domain, boundary lipid domain, and trapped lipid domain (lipids in protein aggregates). The amount of boundary and trapped lipids was greater in intact nuclear membranes than in cortical membranes. The properties of intact membranes were compared with the organization and properties of lens lipid membranes made of the total lipid extracts from the lens cortex or nucleus. In cortical lens lipid membranes, only one homogenous environment was detected, which was designated as a bulk lipid domain (phospholipid bilayer saturated with cholesterol). Lens lipid membranes prepared from the lens nucleus possessed two domains, assigned as a bulk lipid domain and a cholesterol bilayer domain (CBD). In intact nuclear membranes, it was difficult to discriminate the CBD, which was clearly detected in nuclear lens lipid membranes because the OTP measured in the CBD is the same as in the domain formed by trapped lipids. The two domains unique to intact membranes—namely, the domain formed by boundary lipids and the domain formed by trapped lipids—were most likely formed due to the presence of membrane proteins. It is concluded that formation of rigid and practically impermeable domains is enhanced in the lens nucleus, indicating changes in membrane composition that may help to maintain low oxygen concentration in this lens region. PMID:22326289

The Complex Spin State of 103P-Hartley 2: Kinematics and Orientation in Space

NASA Technical Reports Server (NTRS)

Belton, Michael J. S.; Thomas, Peter; Li, Jian-Yang; Williams, Jade; Carcich, Brian; A'Hearn, Michael F.; McLaughlin, Stephanie; Farnham, Tony; McFadden, Lucy; Lisse, Carey M.;

Production cross sections for Lee-Wick massive electromagnetic bosons and for spin-zero and spin-one W bosons at high energies.

NASA Technical Reports Server (NTRS)

Linsker, R.

1972-01-01

Production cross sections for three types of hypothetical particles are calculated in the presented paper. Several (Z, Z') cases were studied corresponding to elastic scattering off protons and neutrons (either free or embedded within a Fermi sea), coherent scattering off a nucleus, and inelastic scattering off a proton (in which case Z' denotes a nucleon resonance or hadronic system in the continuum). Detailed structure-function data are used to improve the accuracy of the inelastic scattering calculation. Results of calculations are given for beam energies between 50 and 10,000 GeV, and masses between 5 and 40 GeV for the massive Lee-Wick spin-1 boson. Cross sections were computed for resonant and semiweak processes. The production cross section of spin-zero weak intermediate bosons was found to be at least one order of magnitude smaller than for spin-1 weak bosons in nearly all regions of interest. The production cross section of spin-zero weak intermediate bosons for inelastic scattering off protons compares with that for elastic scattering in the regions of interest. In the case of massive spin-1 bosons and spin-1 weak intermediates, the main contribution to total production cross section off protons is elastic.

New Global Calculation of Nuclear Masses and Fission Barriers for Astrophysical Applications

NASA Astrophysics Data System (ADS)

Möller, P.; Sierk, A. J.; Bengtsson, R.; Ichikawa, T.; Iwamoto, A.

2008-05-01

The FRDM(1992) mass model [1] has an accuracy of 0.669 MeV in the region where its parameters were determined. For the 529 masses that have been measured since, its accuracy is 0.46 MeV, which is encouraging for applications far from stability in astrophysics. We are developing an improved mass model, the FRDM(2008). The improvements in the calculations with respect to the FRDM(1992) are in two main areas. (1) The macroscopic model parameters are better optimized. By simulation (adjusting to a limited set of now known nuclei) we can show that this actually makes the results more reliable in new regions of nuclei. (2) The ground-state deformation parameters are more accurately calculated. We minimize the energy in a four-dimensional deformation space (ɛ2, V3, V4, V6,) using a grid interval of 0.01 in all 4 deformation variables. The (non-finalized) FRDM (2008-a) has an accuracy of 0.596 MeV with respect to the 2003 Audi mass evaluation before triaxial shape degrees of freedom are included (in progress). When triaxiality effects are incorporated preliminary results indicate that the model accuracy will improve further, to about 0.586 MeV. We also discuss very large-scale fission-barrier calculations in the related FRLDM (2002) model, which has been shown to reproduce very satisfactorily known fission properties, for example barrier heights from 70Se to the heaviest elements, multiple fission modes in the Ra region, asymmetry of mass division in fission and the triple-humped structure found in light actinides. In the superheavy region we find barriers consistent with the observed half-lives. We have completed production calculations and obtain barrier heights for 5254 nuclei heavier than A = 170 for all nuclei between the proton and neutron drip lines. The energy is calculated for 5009325 different shapes for each nucleus and the optimum barrier between ground state and separated fragments is determined by use of an ``immersion'' technique.

Sub-barrier quasifission in heavy element formation reactions with deformed actinide target nuclei

NASA Astrophysics Data System (ADS)

Hinde, D. J.; Jeung, D. Y.; Prasad, E.; Wakhle, A.; Dasgupta, M.; Evers, M.; Luong, D. H.; du Rietz, R.; Simenel, C.; Simpson, E. C.; Williams, E.

2018-02-01

Background: The formation of superheavy elements (SHEs) by fusion of two massive nuclei is severely inhibited by the competing quasifission process. Low excitation energies favor SHE survival against fusion-fission competition. In "cold" fusion with spherical target nuclei near 208Pb, SHE yields are largest at beam energies significantly below the average capture barrier. In "hot" fusion with statically deformed actinide nuclei, this is not the case. Here the elongated deformation-aligned configurations in sub-barrier capture reactions inhibits fusion (formation of a compact compound nucleus), instead favoring rapid reseparation through quasifission. Purpose: To determine the probabilities of fast and slow quasifission in reactions with prolate statically deformed actinide nuclei, through measurement and quantitative analysis of the dependence of quasifission characteristics at beam energies spanning the average capture barrier energy. Methods: The Australian National University Heavy Ion Accelerator Facility and CUBE fission spectrometer have been used to measure fission and quasifission mass and angle distributions for reactions with projectiles from C to S, bombarding Th and U target nuclei. Results: Mass-asymmetric quasifission occurring on a fast time scale, associated with collisions with the tips of the prolate actinide nuclei, shows a rapid increase in probability with increasing projectile charge, the transition being centered around projectile atomic number ZP=14 . For mass-symmetric fission events, deviations of angular anisotropies from expectations for fusion fission, indicating a component of slower quasifission, suggest a similar transition, but centered around ZP˜8 . Conclusions: Collisions with the tips of statically deformed prolate actinide nuclei show evidence for two distinct quasifission processes of different time scales. Their probabilities both increase rapidly with the projectile charge. The probability of fusion can be severely suppressed by these two quasifission processes, since the sub-barrier heavy element yield is likely to be determined by the product of the probabilities of surviving each quasifission process.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ota, S.; Burke, J. T.; Casperson, R. J.

Here, the effect of the production mechanism on the decay of a compound nucleus is investigated. The nucleus 90Zr was produced by three different reactions, namely 90Zr (p,p') 90Zr, 91Zr (p,d) 90Zr, and 92Zr (p,t) 90Zr , which served as surrogate reactions for 89Zr (n,γ). The spin-parity (J π) distributions of the states populated by these reactions were studied to investigate the surrogate reaction approach, which aims at indirectly determining cross sections for compound-nuclear reactions involving unstable targets such as 89Zr. Discrete γ rays, associated with transitions in 90Zr and 89Zr, were measured in coincidence with light ions for scatteringmore » angles of 25°–60° and 90Zr excitation energies extending above the neutron separation energy. The measured transition systematics were used to gain insights into the J π distributions of 90Zr. The 90Zr (p,p') reaction was found to produce fewer γ rays associated with transitions involving high spin states (J = 6–8 ℏ) than the other two reactions, suggesting that inelastic scattering preferentially populates states in 90Zr that have lower spins than those populated in the transfer reactions investigated. The γ-ray production was also observed to vary by factors of 2–3 with the angle at which the outgoing particle was detected. These findings are relevant to the application of the surrogate reaction approach.« less

On the dynamics of fission of hot nuclei

NASA Astrophysics Data System (ADS)

Fröbrich, P.

2007-05-01

In this contribution I take the opportunity to address some points which are in my opinion not in a satisfactory state in the dynamical description of fission of hot nuclei. The focus is on relatively light systems where Bohr's hypothesis on the independence of the fusion and subsequent fission processes is valid, but my remarks are also of relevance to attempts to describe the complete fusion-fission process in a unified way, when quasi-fission channels compete in heavier systems and quantal effects may be of increasing importance in particular when considering low temperatures. There is no doubt that the most adequate dynamical description of the fusion-fission process is obtained by solving multi-dimensional Langevin equations to which a Monte Carlo treatment for the evaporation of light (n, p, α, γ) particles is coupled. However, there is less agreement about the input quantities which enter the description. In the review article [P. Fröbrich, I.I. Gontchar, Phys. Rep. 292, 131 (1998)], we deal mainly with an overdamped Langevin dynamics along the fission coordinate which goes over to an appropriately modified statistical model when a stationary regime with respect to the fission mode is reached. The main ingredient is a phenomenological (deformation-dependent, temperature-independent) friction force, which is invented in such a way that it allows a description of a multitude of experimental data in a universal way (i.e. with the same set of parameters). The main success was a systematic simultaneous description of fission or survival probabilities and prescission neutron multiplicities [P. Fröbrich, I.I. Gontchar, N.D. Mavlitov, Nucl. Phys. A 556, 261 (1993)]. This is not possible in any statistical model. The model describes successfully many other data for systems that develop over a completely equilibrated compound nucleus; see Ref. [P. Fröbrich, I.I. Gontchar, Phys. Rep. 292, 131 (1998)] and references therein. It deals with: fission (survival) probabilities prescission neutron multiplicities and spectra prescission charged particle multiplicities and spectra prescission γ-multiplicities and spectra evaporation residue cross sections fission time distributions temperatures at scission fission fragment angular distributions The results above are obtained with the Ito-discretization of the Langevin equation and might lead to some modifications when using the Klimontovich [Yu.L. Klimontovich, Usp. Fiz. Nauk. 37, 737 (1994)] discretization, which is claimed to be more physical [A.E. Gettinger, I.I. Gontchar, J. Phys. G: Nucl. Part. Phys. 26, 347 (2000)]. A satisfactory description of the measured correlation between the kinetic energy distribution and prescission neutron multiplicities could only be obtained when the mass asymmetry degree of freedom is included in the Langevin theory [P.N. Nadtochy, G.D. Adeev, A.V. Karpov, Phys. Rev. C 65, 064615 (2002)], thus generalizing the two-dimensional not overdamped Langevin models of Refs. [G.R. Tillack, R. Reif, A. Schülcke, P. Fröbrich, H.J. Krappe, H.G. Reusch, Phys. Lett. B 296, 296 (1992)] and [T. Wada, Y. Abe, N. Carjan, Phys. Rev. Lett. 70, 3528 (1993)]. A recent article analysing the mass distribution of fission fragments is [E.G. Ryabov, A.V. Karpov, G.D. Adeev, Nucl. Phys. A 765, 39 (2006)]. The first important point I want to stress is that the driving force of a hot system is not simply the negative gradient of the conservative potential but should contain a thermodynamical correction which is not taken into account in a number of publications.

Fragmentation dynamics of the ethyl bromide and ethyl iodide cations: a velocity-map imaging study.

PubMed

Gardiner, Sara H; Karsili, Tolga N V; Lipciuc, M Laura; Wilman, Edward; Ashfold, Michael N R; Vallance, Claire

2014-02-07

The photodissociation dynamics of ethyl bromide and ethyl iodide cations (C2H5Br(+) and C2H5I(+)) have been studied. Ethyl halide cations were formed through vacuum ultraviolet (VUV) photoionization of the respective neutral parent molecules at 118.2 nm, and were photolysed at a number of ultraviolet (UV) photolysis wavelengths, including 355 nm and wavelengths in the range from 236 to 266 nm. Time-of-flight mass spectra and velocity-map images have been acquired for all fragment ions and for ground (Br) and spin-orbit excited (Br*) bromine atom products, allowing multiple fragmentation pathways to be investigated. The experimental studies are complemented by spin-orbit resolved ab initio calculations of cuts through the potential energy surfaces (along the RC-Br/I stretch coordinate) for the ground and first few excited states of the respective cations. Analysis of the velocity-map images indicates that photoexcited C2H5Br(+) cations undergo prompt C-Br bond fission to form predominantly C2H5(+) + Br* products with a near-limiting 'parallel' recoil velocity distribution. The observed C2H3(+) + H2 + Br product channel is thought to arise via unimolecular decay of highly internally excited C2H5(+) products formed following radiationless transfer from the initial excited state populated by photon absorption. Broadly similar behaviour is observed in the case of C2H5I(+), along with an additional energetically accessible C-I bond fission channel to form C2H5 + I(+) products. HX (X = Br, I) elimination from the highly internally excited C2H5X(+) cation is deemed the most probable route to forming the C2H4(+) fragment ions observed from both cations. Finally, both ethyl halide cations also show evidence of a minor C-C bond fission process to form CH2X(+) + CH3 products.

Investigation of 124Xe nuclear structure with the 8Pi spectrometer at TRIUMF-ISAC

NASA Astrophysics Data System (ADS)

Radich, Allison; Garrett, P.; Jigmeddorj, B.; Michetti-Wilson, J.; Diaz Varela, A.; Hadinia, B.; Bianco, L.; Wong, J.; Chagnon-Lessard, S.; Dunlop, R.; Finlay, P.; Laffoley, A.; Leach, K. G.; Rand, E.; Sumithrarachchi, C.; Svennson, C. E.; Wood, J. L.; Yates, S. W.; Andreoiu, C.; Starosta, K.; Cross, D.; Garnsworthy, A. B.; Hackman, G.; Ball, G.; Triambak, S.

2013-10-01

The 124Xe nucleus has been thought to obey O(6) symmetry but a recent Coulomb excitation study has found that while O(5) may be preserved, O(6) appears to be badly broken. To further characterize the structure of this nucleus, a beta-decay experiment was performed at the TRIUMF-ISAC facility. A beam of radioactive 124Cs at a rate of 9.8 × 107 ions/s was implanted at the center of the 8Pi spectrometer where it underwent β + /EC decay into stable 124Xe. High-statistics gamma-gamma coincidence measurements have been analyzed to add to the level scheme of 124Xe, which has been extended considerably. The high statistics data set has revealed a new decay branch from a 124Cs high-spin isomer as well as several very-weak transitions between low-spin states in 124Xe. Branching ratios and B(E2) transition strengths have been calculated for the updated level scheme. The results will be important in determining collective properties and nuclear structure of the 124Xe.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hattawy, M.; Baltzell, N. A.; Dupré, R.

We report on the first measurement of the beam-spin asymmetry in the exclusive process of coherent deeply virtual Compton scattering off a nucleus. The experiment uses the 6 GeV electron beam from the Continuous Electron Beam Accelerator Facility (CEBAF) accelerator at Jefferson Lab incident on a pressurized He-4 gaseous target placed in front of the CEBAF Large Acceptance Spectrometer (CLAS). The scattered electron is detected by CLAS and the photon by a dedicated electromagnetic calorimeter at forward angles. To ensure the exclusivity of the process, a specially designed radial time projection chamber is used to detect the recoiling He-4 nuclei.more » We measure beam-spin asymmetries larger than those observed on the free proton in the same kinematic domain. From these, we are able to extract, in a model-independent way, the real and imaginary parts of the only He-4 Compton form factor, HA. This first measurement of coherent deeply virtual Compton scattering on the He-4 nucleus, with a fully exclusive final state via nuclear recoil tagging, leads the way toward 3D imaging of the partonic structure of nuclei.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hattawy, M.; Baltzell, N. A.; Dupré, R.

Here, we report on the first measurement of the beam-spin asymmetry in the exclusive process of coherent deeply virtual Compton scattering off a nucleus. The experiment used the 6 GeV electron beam from the CEBAF accelerator at Jefferson Lab incident on a pressurizedmore » $^4$He gaseous target placed in front of the CEBAF Large Acceptance Spectrometer (CLAS). The scattered electron was detected by CLAS and the photon by a dedicated electromagnetic calorimeter at forward angles. To ensure the exclusivity of the process, a specially designed radial time projection chamber was used to detect the recoiling $^4$He nuclei. We measured beam-spin asymmetries larger than those observed on the free proton in the same kinematic domain. From these, we were able to extract, in a model-independent way, the real and imaginary parts of the only $^4$He Compton form factor, $$\\cal H_A$$. This first measurement of coherent deeply virtual Compton scattering on the $^4$He nucleus, with a fully exclusive final state via nuclear recoil tagging, leads the way toward 3D imaging of the partonic structure of nuclei.« less

Identification of yrast high-K intrinsic states in {sup 188}Os

DOE Office of Scientific and Technical Information (OSTI.GOV)

Modamio, V.; Jungclaus, A.; Instituto de Estructura de la Materia, CSIC, Serrano 113bis, E-28006 Madrid

2009-02-15

The high-spin structure of the Z=76 nucleus {sup 188}Os has been studied using the incomplete fusion reaction {sup 7}Li+{sup 186}W. A K{sup {pi}}=10{sup +} band has been established up to spin (24{sup +}) and its crossing with the ground-state band has been studied. In addition, intrinsic high-K states have been identified and on top of two of them, K{sup {pi}}=7{sup -} and K{sup {pi}}=10{sup -}, regular bands have been observed. The K{sup {pi}}=16{sup +} and K{sup {pi}}=18{sup +} states are yrast whereas the K{sup {pi}}=14{sup +} level lies only 33 keV above the yrast line and decays with a lowmore » reduced hindrance of f{sub {nu}}<1.3 to the ground-state band ({delta}K=14). The results are discussed by means of a systematic comparison with the even-even neighboring nucleus {sup 186}Os. Configuration-constrained multiquasiparticle potential-energy-surface calculations have been performed to identify the configurations of multiquasiparticle states.« less

Nuclear Spin Dependent Parity Violation in Diatomic Molecules

NASA Astrophysics Data System (ADS)

Cahn, Sidney; Altuntas, Emine; Ammon, Jeffrey; Demille, David

2015-10-01

Nuclear spin-dependent parity violation (NSD-PV) effects arise from the exchange of the Z0 boson between electrons and the nucleus and from the interaction of electrons with the nuclear anapole moment, a parity-odd magnetic moment. The anapole moment grows as A2/3 of the nucleus,while the Z0 coupling is independent of A. We study NSD-PV effects using diatomic molecules, where signals are dramatically amplified by bringing rotational levels of opposite parity close to degeneracy in a strong magnetic field. Using a Stark-interference technique, we measure the NSD-PV interaction matrix element. We present results that demonstrate statistical sensitivity to NSD-PV effects surpassing that of any previous atomic parity violation measurement, using the test system 138Ba19F. We also discuss improvements on investigations of systematics due to non-reversing stray E-fields, Enr together with B-field inhomogeneities, and short-term prospects for measuring the nuclear anapole moment of 137Ba. In the long term, our technique is sufficiently general and sensitive to enable measurements across a broad range of nuclei.

Molecular dynamics simulation of thermal transport in UO 2 containing uranium, oxygen, and fission-product defects

DOE PAGES

Liu, Xiang -Yang; Cooper, Michael William D.; McClellan, Kenneth James; ...

2016-10-25

Uranium dioxide (UO 2) is the most commonly used fuel in light-water nuclear reactors and thermal conductivity controls the removal of heat produced by fission, thereby governing fuel temperature during normal and accident conditions. The use of fuel performance codes by the industry to predict operational behavior is widespread. A primary source of uncertainty in these codes is thermal conductivity, and optimized fuel utilization may be possible if existing empirical models are replaced with models that incorporate explicit thermal-conductivity-degradation mechanisms during fuel burn up. This approach is able to represent the degradation of thermal conductivity due to each individual defectmore » type, rather than the overall burn-up measure typically used, which is not an accurate representation of the chemical or microstructure state of the fuel that actually governs thermal conductivity and other properties. To generate a mechanistic thermal conductivity model, molecular dynamics (MD) simulations of UO 2 thermal conductivity including representative uranium and oxygen defects and fission products are carried out. These calculations employ a standard Buckingham-type interatomic potential and a potential that combines the many-body embedded-atom-method potential with Morse-Buckingham pair potentials. Potential parameters for UO 2+x and ZrO 2 are developed for the latter potential. Physical insights from the resonant phonon-spin-scattering mechanism due to spins on the magnetic uranium ions are introduced into the treatment of the MD results, with the corresponding relaxation time derived from existing experimental data. High defect scattering is predicted for Xe atoms compared to that of La and Zr ions. Uranium defects reduce the thermal conductivity more than oxygen defects. For each defect and fission product, scattering parameters are derived for application in both a Callaway model and the corresponding high-temperature model typically used in fuel-performance codes. The model is validated by comparison to low-temperature experimental measurements on single-crystal hyperstoichiometric UO 2+x samples and high-temperature literature data. Furthermore, this work will enable more accurate fuel-performance simulations and will extend to new fuel types and operating conditions, all of which improve the fuel economics of nuclear energy and maintain high fuel reliability and safety.« less

Molecular dynamics simulation of thermal transport in UO 2 containing uranium, oxygen, and fission-product defects

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Xiang -Yang; Cooper, Michael William D.; McClellan, Kenneth James

Uranium dioxide (UO 2) is the most commonly used fuel in light-water nuclear reactors and thermal conductivity controls the removal of heat produced by fission, thereby governing fuel temperature during normal and accident conditions. The use of fuel performance codes by the industry to predict operational behavior is widespread. A primary source of uncertainty in these codes is thermal conductivity, and optimized fuel utilization may be possible if existing empirical models are replaced with models that incorporate explicit thermal-conductivity-degradation mechanisms during fuel burn up. This approach is able to represent the degradation of thermal conductivity due to each individual defectmore » type, rather than the overall burn-up measure typically used, which is not an accurate representation of the chemical or microstructure state of the fuel that actually governs thermal conductivity and other properties. To generate a mechanistic thermal conductivity model, molecular dynamics (MD) simulations of UO 2 thermal conductivity including representative uranium and oxygen defects and fission products are carried out. These calculations employ a standard Buckingham-type interatomic potential and a potential that combines the many-body embedded-atom-method potential with Morse-Buckingham pair potentials. Potential parameters for UO 2+x and ZrO 2 are developed for the latter potential. Physical insights from the resonant phonon-spin-scattering mechanism due to spins on the magnetic uranium ions are introduced into the treatment of the MD results, with the corresponding relaxation time derived from existing experimental data. High defect scattering is predicted for Xe atoms compared to that of La and Zr ions. Uranium defects reduce the thermal conductivity more than oxygen defects. For each defect and fission product, scattering parameters are derived for application in both a Callaway model and the corresponding high-temperature model typically used in fuel-performance codes. The model is validated by comparison to low-temperature experimental measurements on single-crystal hyperstoichiometric UO 2+x samples and high-temperature literature data. Furthermore, this work will enable more accurate fuel-performance simulations and will extend to new fuel types and operating conditions, all of which improve the fuel economics of nuclear energy and maintain high fuel reliability and safety.« less

Structure of the exotic He 9 nucleus from the no-core shell model with continuum

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vorabbi, Matteo; Calci, Angelo; Navratil, Petr

2018-03-13

Here, the exotic 9He nucleus, which presents one of the most extreme neutron-to-proton ratios, belongs to the N = 7 isotonic chain famous for the phenomenon of ground-state parity inversion with decreasing number of protons. Consequently, it would be expected to have an unnatural (positive) parity ground state similar to 11Be and 10Li. Despite many experimental and theoretical investigations, its structure remains uncertain. Apart from the fact that it is unbound, other properties including the spin and parity of its ground state, and the very existence of additional low-lying resonances are still a matter of debate

Tidal waves in 102Pd: a rotating condensate of multiple d bosons.

PubMed

Ayangeakaa, A D; Garg, U; Caprio, M A; Carpenter, M P; Ghugre, S S; Janssens, R V F; Kondev, F G; Matta, J T; Mukhopadhyay, S; Patel, D; Seweryniak, D; Sun, J; Zhu, S; Frauendorf, S

2013-03-08

Low-lying collective excitations in even-even vibrational and transitional nuclei may be described semiclassically as quadrupole running waves on the surface of the nucleus ("tidal waves"), and the observed vibrational-rotational behavior can be thought of as resulting from a rotating condensate of interacting d bosons. These concepts have been investigated by measuring lifetimes of the levels in the yrast band of the (102)Pd nucleus with the Doppler shift attenuation method. The extracted B(E2) reduced transition probabilities for the yrast band display a monotonic increase with spin, in agreement with the interpretation based on rotation-induced condensation of aligned d bosons.

Nuclear Forensics using Gamma-ray Spectroscopy

NASA Astrophysics Data System (ADS)

Norman, E. B.

2016-09-01

Much of George Dracoulis's research career was devoted to utilising gamma-ray spectroscopy in fundamental studies in nuclear physics. This same technology is useful in a wide range of applications in the area of nuclear forensics. Over the last several years, our research group has made use of both high- and low-resolution gamma-ray spectrometers to: identify the first sample of plutonium large enough to be weighed; determine the yield of the Trinity nuclear explosion; measure fission fragment yields as a function of target nucleus and neutron energy; and observe fallout in the U. S. from the Fukushima nuclear reactor accident.

Loss of endocytic capacity in aging Paramecium. The importance of cytoplasmic organelles

PubMed Central

1976-01-01

Aged cells have significantly fewer food vacuoles and ingest fewer bacteria than young cells. Loss of food vacuoles was explained by a decreasing difference in the food vacuole formation and excretion rates; the formation rate declined more rapidly than the excretion rate, approaching equivalence at 160 fissions, when the proportion of cells with no food vacuoles, in the presence of excess food, abruptly increased. A model for cellular aging is presented in which control of organelle numbers and cyclical interactions between the nucleus and cytoplasm may be of critical importance. PMID:993263

First evidence of γ collectivity close to the doubly magic core Sn 132

DOE Office of Scientific and Technical Information (OSTI.GOV)

Urban, W.; Sieja, K.; Rząca-Urban, T.

2016-03-01

The Te-138 and Xe-140 nuclei have been reinvestigated using prompt gamma-ray data from spontaneous fission of Cm-248, collected with the EUROGAM2 Ge array. gamma bands have been identified in both nuclei. The gamma band observed in Te-138, a nucleus with only six valence nucleons, indicates the presence of collectivity very close to the doubly magic Sn-132 core. Such band is even more pronounced in Xe-140, the N = 86 isotone of Te-138. The newly observed bands are interpreted within the shell model, which reproduce well the. collectivity at N = 86.

Structure of the exotic 9He nucleus from the no-core shell model with continuum

NASA Astrophysics Data System (ADS)

Vorabbi, Matteo; Calci, Angelo; Navrátil, Petr; Kruse, Michael K. G.; Quaglioni, Sofia; Hupin, Guillaume

2018-03-01

Background: The exotic 9He nucleus, which presents one of the most extreme neutron-to-proton ratios, belongs to the N =7 isotonic chain famous for the phenomenon of ground-state parity inversion with decreasing number of protons. Consequently, it would be expected to have an unnatural (positive) parity ground state similar to 11Be and 10Li. Despite many experimental and theoretical investigations, its structure remains uncertain. Apart from the fact that it is unbound, other properties including the spin and parity of its ground state, and the very existence of additional low-lying resonances are still a matter of debate. Purpose: In this work, we study the properties of 9He by analyzing the n +8He continuum in the context of the ab initio no-core shell model with continuum (NCSMC) formalism with chiral nucleon-nucleon interactions as the only input. Methods: The NCSMC is a state-of-the-art approach for the ab initio description of light nuclei. With its capability to predict properties of bound states, resonances, and scattering states in a unified framework, the method is particularly well suited for the study of unbound nuclei such as 9He. Results: Our analysis produces an unbound 9He nucleus. Two resonant states are found at the energies of ˜1 and ˜3.5 MeV, respectively, above the n +8He breakup threshold. The first state has a spin-parity assignment of Jπ=1/2 - and can be associated with the ground state of 9He, while the second, broader state has a spin parity of 3/2 -. No resonance is found in the 1/2 + channel, only a very weak attraction. Conclusions: We find that the 9He ground-state resonance has a negative parity and thus breaks the parity-inversion mechanism found in the 11Be and 10Li nuclei of the same N =7 isotonic chain.

Spin properties of supermassive black holes with powerful outflows

NASA Astrophysics Data System (ADS)

Daly, Ruth. A.

2016-05-01

Relationships between beam power and accretion disc luminosity are studied for a sample of 55 high excitation radio galaxies (HERG), 13 low excitation radio galaxies (LERG), and 29 radio loud quasars (RLQ) with powerful outflows. The ratio of beam power to disc luminosity tends to be high for LERG, low for RLQ, and spans the full range of values for HERG. Writing general expressions for the disc luminosity and beam power and applying the empirically determined relationships allows a function that parametrizes the spins of the holes to be estimated. Interestingly, one of the solutions that is consistent with the data has a functional form that is remarkably similar to that expected in the generalized Blandford-Znajek model with a magnetic field that is similar in form to that expected in magnetically arrested disk (MAD) and advection-dominated accretion flow (ADAF) models. Values of the spin function, obtained independent of specific outflow models, suggest that spin and active galactic nucleus type are not related for these types of sources. The spin function can be used to solve for black hole spin in the context of particular outflow models, and one example is provided.

Storing quantum information for 30 seconds in a nanoelectronic device.

PubMed

Muhonen, Juha T; Dehollain, Juan P; Laucht, Arne; Hudson, Fay E; Kalra, Rachpon; Sekiguchi, Takeharu; Itoh, Kohei M; Jamieson, David N; McCallum, Jeffrey C; Dzurak, Andrew S; Morello, Andrea

2014-12-01

The spin of an electron or a nucleus in a semiconductor naturally implements the unit of quantum information--the qubit. In addition, because semiconductors are currently used in the electronics industry, developing qubits in semiconductors would be a promising route to realize scalable quantum information devices. The solid-state environment, however, may provide deleterious interactions between the qubit and the nuclear spins of surrounding atoms, or charge and spin fluctuations arising from defects in oxides and interfaces. For materials such as silicon, enrichment of the spin-zero (28)Si isotope drastically reduces spin-bath decoherence. Experiments on bulk spin ensembles in (28)Si crystals have indeed demonstrated extraordinary coherence times. However, it remained unclear whether these would persist at the single-spin level, in gated nanostructures near amorphous interfaces. Here, we present the coherent operation of individual (31)P electron and nuclear spin qubits in a top-gated nanostructure, fabricated on an isotopically engineered (28)Si substrate. The (31)P nuclear spin sets the new benchmark coherence time (>30 s with Carr-Purcell-Meiboom-Gill (CPMG) sequence) of any single qubit in the solid state and reaches >99.99% control fidelity. The electron spin CPMG coherence time exceeds 0.5 s, and detailed noise spectroscopy indicates that--contrary to widespread belief--it is not limited by the proximity to an interface. Instead, decoherence is probably dominated by thermal and magnetic noise external to the device, and is thus amenable to further improvement.

Histone H4 acetylation required for chromatin decompaction during DNA replication.

PubMed

Ruan, Kun; Yamamoto, Takaharu G; Asakawa, Haruhiko; Chikashige, Yuji; Kimura, Hiroshi; Masukata, Hisao; Haraguchi, Tokuko; Hiraoka, Yasushi

2015-07-30

Faithful DNA replication is a prerequisite for cell proliferation. Several cytological studies have shown that chromosome structures alter in the S-phase of the cell cycle. However, the molecular mechanisms behind the alteration of chromosome structures associated with DNA replication have not been elucidated. Here, we investigated chromatin structures and acetylation of specific histone residues during DNA replication using the meiotic nucleus of the fission yeast Schizosaccharomyces pombe. The S. pombe meiotic nucleus provides a unique opportunity for measuring the levels of compaction of chromatin along the chromosome in a defined orientation. By direct measurement of chromatin compaction in living cells, we demonstrated that decompaction of chromatin occurs during meiotic DNA replication. This chromatin decompaction was suppressed by depletion of histone acetyltransferase Mst1 or by arginine substitution of specific lysine residues (K8 and K12) of histone H4. These results suggest that acetylation of histone H4 residues K8 and K12 plays a critical role in loosening chromatin structures during DNA replication.

Meiotic Nuclear Oscillations Are Necessary to Avoid Excessive Chromosome Associations.

PubMed

Chacón, Mariola R; Delivani, Petrina; Tolić, Iva M

2016-11-01

Pairing of homologous chromosomes is a crucial step in meiosis, which in fission yeast depends on nuclear oscillations. However, how nuclear oscillations help pairing is unknown. Here, we show that homologous loci typically pair when the spindle pole body is at the cell pole and the nucleus is elongated, whereas they unpair when the spindle pole body is in the cell center and the nucleus is round. Inhibition of oscillations demonstrated that movement is required for initial pairing and that prolonged association of loci leads to mis-segregation. The double-strand break marker Rec25 accumulates in elongated nuclei, indicating that prolonged chromosome stretching triggers recombinatory pathways leading to mis-segregation. Mis-segregation is rescued by overexpression of the Holliday junction resolvase Mus81, suggesting that prolonged pairing results in irresolvable recombination intermediates. We conclude that nuclear oscillations exhibit a dual role, promoting initial pairing and restricting the time of chromosome associations to ensure proper segregation. Copyright © 2016 The Author(s). Published by Elsevier Inc. All rights reserved.

Laser nanosurgery and manipulation in living cells

NASA Astrophysics Data System (ADS)

Sacconi, Leonardo; Tolic-Norrelykke, Iva M.; Antolini, Renzo; Pavone, Francesco S.

2005-03-01

We present a combination of nonlinear microscopy, laser nanosurgery and optical trapping applied to the 3D imaging and manipulation of intracellular structures in live cells. We use Titanium-sapphire laser pulses for a combined nonlinear microscopy and nanosurgery on microtubules tagged with green fluorescent protein (GFP) in fission yeast. The same laser source is also used to trap small round lipid droplets naturally present in the cell. The trapped droplets are used as handles to exert a pushing force on the nucleus, allowing for a displacement of the nucleus away from its normal position in the center of the cell. We show that nonlinear nanosurgery and optical manipulation can be performed with sub-micrometer precision and without visible collateral damage to the cell. We present this combination as an important tool in cell biology for the manipulation of specific structures in alternative to genetic methods or chemical agents. This technique can be applied to several fundamental problems in cell biology, including the study of dynamics processes in cell division.

Many-body kinetics of dynamic nuclear polarization by the cross effect

NASA Astrophysics Data System (ADS)

Karabanov, A.; Wiśniewski, D.; Raimondi, F.; Lesanovsky, I.; Köckenberger, W.

2018-03-01

Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating nonthermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance is cross-effect DNP, which involves the interaction of two coupled electrons with the nuclear spin ensemble. Here we develop a theory for this important DNP mechanism and show that the nonequilibrium nuclear polarization buildup is effectively driven by three-body incoherent Markovian dissipative processes involving simultaneous state changes of two electrons and one nucleus. We identify different parameter regimes for effective polarization transfer and discuss under which conditions the polarization dynamics can be simulated by classical kinetic Monte Carlo methods. Our theoretical approach allows simulations of the polarization dynamics on an individual spin level for ensembles consisting of hundreds of nuclear spins. The insight obtained by these simulations can be used to find optimal experimental conditions for cross-effect DNP and to design tailored radical systems that provide optimal DNP efficiency.

Fission and Properties of Neutron-Rich Nuclei

NASA Astrophysics Data System (ADS)

Hamilton, Joseph H.; Ramayya, A. V.; Carter, H. K.

2008-08-01

Opening session. Nuclear processes in stellar explosions / M. Wiescher. In-beam [symbol]-ray spectroscopy of neutron-rich nuclei at NSCL / A. Gade -- Nuclear structure I. Shell-model structure of neutron-rich nuclei beyond [symbol]Sn / A. Covello ... [et al.]. Shell structure and evolution of collectivity in nuclei above the [symbol]Sn core / S. Sarkar and M. S. Sarkar. Heavy-ion fusion using density-constrained TDHF / A. S. Umar and V. E. Oberacker. Towards an extended microscopic theory for upper-fp shell nuclei / K. P. Drumev. Properties of the Zr and Pb isotopes near the drip-line / V. N. Tarasov ... [et al.]. Identification of high spin states in [symbol] Cs nuclei and shell model calculations / K. Li ... [et al.]. Recent measurements of spherical and deformed isomers using the Lohengrin fission-fragment spectrometer / G. S. Simpson ... [et al.] -- Nuclear structure II. Nuclear structure investigation with rare isotope spectroscopic investigations at GSI / P. Boutachkov. Exploring the evolution of the shell structures by means of deep inelastic reactions / G. de Anaelis. Probing shell closures in neutron-rich nuclei / R. Krücken for the S277 and REX-ISOLDEMINIBALL collaborations. Structure of Fe isotopes at the limits of the pf-shell / N. Hoteling ... [et al.]. Spectroscopy of K isomers in shell-stabilized trans-fermium nuclei / S. K. Tandel ... [et al.] -- Radioactive ion beam facilities. SPIRAL2 at GANIL: a world leading ISOL facility for the next decade / S. Gales. New physics at the International Facility for Antiproton and Ion Research (FAIR) next to GSI / I. Augustin ... [et al.]. Radioactive beams from a high powered ISOL system / A. C. Shotter. RlKEN RT beam factory / T. Motobayashi. NSCL - ongoing activities and future perspectives / C. K. Gelbke. Rare isotope beams at Argonne / W. F. Henning. HRIBF: scientific highlights and future prospects / J. R. Beene. Radioactive ion beam research done in Dubna / G. M. Ter-Akopian ... [et al.] -- Fission I. Fission-fragment spectroscopy with STEFF / A. G. Smith ... [et al.]. Gamma ray multiplicity of [symbol]Cf spontaneous fission using LiBerACE / D. L. Bleuel ... [et al.]. Excitation energy dependence of fragment mass and total kinetic energy distributions in proton-induced fission of light actinides / I. Nishinaka ... [et al.]. A dynamical calculation of multi-modal nuclear fission / T. Wada and T. Asano. Structure of fission potential energy surfaces in ten-dimensional spaces / V. V. Pashkevich, Y. K Pyatkov and A. V. Unzhakova. A possible enhancement of nuclear fission in scattering with low energy charged particles / V. Gudkov. Dynamical multi-break processes in the [symbol]Sn + [symbol]Ni system at 35 MeV/Nucleon / M. Papa and ISOSPIN-RE VERSE collaboration -- New experimental techniques. MTOF - a high resolution isobar separator for studies of exotic decays / A. Piechaczek ... [et al.]. Development of ORRUBA: a silicon array for the measurement of transfer reactions in inverse kinematics / S. D. Pain ... [et al.]. Indian national gamma array: present & future / R. K. Bhowmik. Absolute intensities of [symbol] rays emitted in the decay of [symbol]U / H. C. Griffin -- Superheavy elements theory and experiments / M. G. Itkis ... [et al.]. Study of superheavy elements at SHIP / S. Hofinann. Heaviest nuclei from [symbol]Ca-induced reactions / Yu. Ts. Oaanessian. Superheavy nuclei and giant nuclear systems / W. Greiner and V. Zagrebaev. Fission approach to alpha-decay of superheavy nuclei / D.N. Poenaru and W. Greiner. Superheavy elements in the Magic Islands / C. Samanta. Relativistic mean field studies of superheavy nuclei / A. V. Afanas jev. Understanding the synthesis of the heaviest nuclei / W. Loveland -- Mass measurements and g-factors. G factor measurements in neutron-rich [symbol]Cf fission fragments, measured using the gammasphere array / R. Orlandi ... [et al.]. Technique for measuring angular correlations and g-factors in neutron rich nuclei produced by the spontaneous fission of [symbol]Cf / A. V. Daniel ... [et al.]. Magnetic moment measurements in a radioactive beam environment / N. Benczer-Koller and G. Kumbartzki. g-Factor measurements of picosecond states: opportunities and limitations of the recoil-in-vacuum method / N. J. Stone ... [et al.]. Precision mass measurements and trap-assisted spectroscopy of fission products from Ni to Pd / A. Jokinen -- Fission II. Fission research at IRMM / F.-J. Hambsch. Fission yield measurements at the IGISOL facility with JYFLTRAP / H. Penttilä ... [et al.]. Fission of radioactive beams and dissipation in nuclear matter / A. Heinz (for the CHARMS collaboration). Fission of [symbol]U at 80 MeVlu and search for new neutron-rich isotopes / C.M. Folden, III ... [et al.]. Measurement of the average energy and multiplicity of prompt-fission neutrons and gamma rays from [symbol], [symbol], and [symbol] for incident neutron energies of 1 to 200 MeV / R. C. Haight ... [et al.]. Fission measurements with DANCE / M. Jandel ... [et al.]. Measured and calculated neutron-induced fission cross sections of [symbol]Pu / F. Tovesson and T. S. Hill. The fission barrier landscape / L. Phair and L. G. Moretto. Fast neutron-induced fission of some actinides and sub-actinides / A. B. Lautev ... [et al.] -- Fission III/Nuclear structure III. Complex structure in even-odd staggering of fission fragment yields / M. Caamāno and F. Rejmund. The surrogate method: past, present and future / S. R. Lesher ... [et al]. Effects of nuclear incompressibility on heavy-ion fusion / H. Esbensen and Ş. Mişicu. High spin states in [symbol]Pm / A. Dhal ... [et al]. Structure of [symbol]Sm, spherical vibrator versus softly deformed rotor / J. B. Gupta -- Astrophysics. Measuring the astrophysical S-factor in plasmas / A. Bonasera ... [et al.]. Is there shell quenching or shape coexistence in Cd isotopes near N = 82? / J. K. Hwang, A. V. Ramayya and J. H. Hamilton. Spectroscopy of neutron-rich palladium and cadmium isostopes near A= 120 / M. A. Stoyer and W. B. Walters -- Nuclear structure IV. First observation of new neutron-rich magnesium, aluminum and silicon isotopes / A. Stolz ... [et al.]. Spectroscopy of [symbol]Na revolution of shell structure with isospin / V. Tripathi ... [et al.]. Rearrangement of proton single particle orbitals in neutron-rich potassium isotopes - spectroscopy of [symbol]K / W. Królas ... [et al.]. Laser spectroscopy and the nature of the shape transition at N [symbol] 60 / B. Cheal ... [et al.]. Study of nuclei near stability as fission fragments following heavy-ion reactions / N. Fotiadis. [symbol]C and [symbol]N: lifetime measurements of their first-excited states / M. Wiedeking ... [et al.] -- Nuclear astrophysics. Isomer spectroscopy near [symbol]Sn - first observation of excited states in [symbol]Cd / M. Pfitzner ... [et al.]. Nuclear masses and what they imply for the structures of neutron rich nuclei / A. Awahamian and A. Teymurazyan. Multiple nucleosynthesis processes in the early universe / F. Montes. Single-neutron structure of neutron-rich nuclei near N = 50 and N = 82 / J. A. Cizewski ... [et al.]. [symbol]Cadmium: ugly duckling or young swan / W. B. Walters ... [et al.] -- Nuclear structure V. Evidence for chiral doublet bands in [symbol]Ru / Y. X. Luo ... [et al.]. Unusual octupole shape deformation terms and K-mixing / J. O. Rasmussen ... [et al.]. Spin assignments, mixing ratios, and g-factors in neutron rich [symbol]Cf fission products / C. Goodin ... [et al.]. Level structures and double [symbol]-bands in [symbol]Mo, [symbol]Mo and [symbol]Ru / S. J. Zhu ... [et al.] -- Nuclear theory. Microscopic dynamics of shape coexistence phenomena around [symbol]Se and [symbol]Kr / N. Hinohara ... [et al.]. Nuclear structure, double beta decay and test of physics beyond the standard model / A. Faessler. Collective modes in elastic nuclear matter / Ş. Mişicu and S. Bastrukov. From N = Z to neutron rich: magnetic moments of Cu isotopes at and above the [symbol]Ni and [symbol]Ni double shell closures - what next? / N. J. Stone, J. R. Stone and U. Köster -- Nuclear structure VI. Decay studies of nuclei near [symbol]Ni / R. Grzywacz. Weakening of the [symbol]Ni core for Z > 28, N > 50? / J. A. Winger ... [et al.]. Coulomb excitation of the odd-A [symbol]Cu isotopes with MINIBALL and REX-ISOLDE / I. Stefanescu ... [et al.]. Neutron single particle states and isomers in odd mass nickel isotopes near [symbol]Ni / M. M. Raiabali ... [et al.]. [symbol] and [symbol]-delayed neutron decay studies of [symbol]Ch at the HRIBF / S. V. Ilvushkin ... [et al.] -- Posters. Properties of Fe, Ni and Zn isotope chains near the drip-line / V. N. Tarasov ... [et al.]. Probing nuclear structure of [symbol]Xe / J. B. Gupta. Shape coexistence in [symbol]Zr and large deformation in [symbol]Zr / J. K. Hwang ... [et al.]. Digital electronics and their application to beta decay spectroscopy / S. N. Liddick, S. Padgett and R. Grzywacz. Nuclear shape and structure in neutron-rich [symbol]Tc / Y. X. Luo ... [et al.]. Speeding up the r-process. Investigation of first forbidden [symbol] decays in N > 50 isotopes near [symbol]Ni / S. Padgett ... [et al.]. Yields of fission products from various actinide targets / E. H. Sveiewski ... [et al.].

Bose-Fermi symmetry in the odd-even gold isotopes

NASA Astrophysics Data System (ADS)

Thomas, T.; Régis, J.-M.; Jolie, J.; Heinze, S.; Albers, M.; Bernards, C.; Fransen, C.; Radeck, D.

2014-05-01

In this work the results of an in-beam experiment on 195Au are presented, yielding new spins, multipole mixing ratios, and new low-lying states essential for the understanding of this nucleus. The positive-parity states from this work together with compiled data from the available literature for 185-199Au are compared to Interacting Boson Fermion Model calculations employing the Spin(6) Bose-Fermi symmetry. The evolution of the parameters for the τ splitting and the J splitting reveals a smooth behavior. Thereby, a common description based on the Bose-Fermi symmetry is found for 189-199Au. Furthermore, the calculated E2 transition strengths are compared to experimental values with fixed effective boson and fermion charges for all odd-even gold isotopes, emphasizing that the Spin(6) Bose-Fermi symmetry is valid for the gold isotopes.

Absence of paired crossing in the positive parity bands of 124Cs

NASA Astrophysics Data System (ADS)

Singh, A. K.; Basu, A.; Nag, Somnath; Hübel, H.; Domscheit, J.; Ragnarsson, I.; Al-Khatib, A.; Hagemann, G. B.; Herskind, B.; Elema, D. R.; Wilson, J. N.; Clark, R. M.; Cromaz, M.; Fallon, P.; Görgen, A.; Lee, I.-Y.; Ward, D.; Ma, W. C.

2018-02-01

High-spin states in 124Cs were populated in the 64Ni(64Ni,p 3 n ) reaction and the Gammasphere detector array was used to measure γ -ray coincidences. Both positive- and negative-parity bands, including bands with chiral configurations, have been extended to higher spin, where a shape change has been observed. The configurations of the bands before and after the alignment are discussed within the framework of the cranked Nilsson-Strutinsky model. The calculations suggest that the nucleus undergoes a shape transition from triaxial to prolate around spin I ≃22 of the positive-parity states. The alignment gain of 8 ℏ , observed in the positive-parity bands, is due to partial alignment of several valence nucleons. This indicates the absence of band crossing due to paired nucleons in the bands.

Total absorption γ -ray spectroscopy of the β -delayed neutron emitters Br 87 , Br 88 , and Rb 94

DOE PAGES

Valencia, E.; Tain, J. L.; Algora, A.; ...

2017-02-21

In this paper, we investigate the decay of 87,88Br and 94Rb using total absorption γ-ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ intensity, so far unobserved in high-resolution γ-ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component formore » 235U fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for γ emission from neutron unbound states populated in the daughter nucleus. The γ branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94Rb, although much smaller, hints of the need to increase the radiative width Γ γ by one order of magnitude. Finally, this increase in Γ γ would lead to a similar increase in the calculated (n, γ) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.« less

Dynamics of 47V* formed in 20Ne + 27Al reaction in view of fusion-fission and DIC mechanism

NASA Astrophysics Data System (ADS)

Grover, Neha; Sharma, Kanishka; Sharma, Manoj K.

2017-12-01

The decay mechanism of 47V* formed in direct kinematics (20Ne + 27Al is investigated within the collective clusterization approach of dynamical cluster decay model (DCM). All calculations are done for quadrupole ( β 2 i -deformed) choice of fragments by taking optimum orientations over a wide range of center of mass energies ( E c. m. ˜ 83-125 MeV). According to the experimental evidence, there is a strong competition between fusion fission (FF) and deep inelastic collision (DIC) in the decay of 47V*, which are recognized as compound nucleus process and non-compound nucleus process, respectively. The decay cross sections of 47V* for both FF and DIC decay modes are addressed using DCM, and are found to be in agreement with the experimental data. It is important to mention that emitting fragments in both these decay channels maintain their homogeneity in terms of charge number, that lies in the region 3 ≤ Z ≤ 9. Hence, all possible isotopes contributing towards 3 ≤ Z ≤ 9 are taken into consideration here. Calculations of both FF and DIC are segregated on the basis of angular momentum windows, where 0 ≤ ℓ ≤ ℓ cr has been taken for FF and ℓ cr < ℓ ≤ ℓ gr for DIC, as the later operates only due to the partial waves near grazing angular momentum. In DIC, preformation probability ( P 0) is divided equally amongst the most favoured outgoing fragments. Moreover, the behavior of fragmentation potential, preformation probability, penetrability and emission time etc. is examined, in order to identify the most favorable isotopes contributing towards FF and DIC.

Fabrication and characterization of carbon-backed thin 208Pb targets.

PubMed

Thakur, Meenu; Dubey, R; Abhilash, S R; Behera, B R; Mohanty, B P; Kabiraj, D; Ojha, Sunil; Duggal, Heena

2016-01-01

Thin carbon-backed isotopically enriched 208 Pb targets were required for our experiment aimed to study the reaction dynamics for 48 Ti +  208 Pb system, populating the near super-heavy nucleus 256 Rf, through mass-energy correlation of the fission fragments. Purity and thickness of the targets are of utmost importance in such studies as these factors have strong influence on the measurement accuracy of mass and energy distribution of fission fragments. 208 Pb targets with thickness ranging from 60 μg/cm 2 to 250 μg/cm 2 have been fabricated in high vacuum environment using physical vapor deposition method. Important points in the method are as follows: • 208 Pb was deposited using resistive heating method, whereas carbon (backing foil) deposition was performed by using the electron beam bombardment technique.•Different characterization techniques such as Particle Induced X-ray Emission (PIXE), Energy Dispersive X-Ray Fluorescence (EDXRF) and Rutherford Backscattering Spectrometry (RBS) were used to assert the purity and thickness of the targets.•These targets have successfully been used to accomplish our experimental objectives.

Helical modes generate antimagnetic rotational spectra in nuclei

NASA Astrophysics Data System (ADS)

Malik, Sham S.

2018-03-01

A systematic analysis of the antimagnetic rotation band using r -helicity formalism is carried out for the first time. The observed octupole correlation in a nucleus is likely to play a role in establishing the antimagnetic spectrum. Such octupole correlations are explained within the helical orbits. In a rotating field, two identical fermions (generally protons) with paired spins generate these helical orbits in such a way that its positive (i.e., up) spin along the axis of quantization refers to one helicity (right-handedness) while negative (down) spin along the same quantization-axis decides another helicity (left-handedness). Since the helicity remains invariant under rotation, therefore, the quantum state of a fermion is represented by definite angular momentum and helicity. These helicity represented states support a pear-shaped structure of a rotating system having z axis as the symmetry axis. A combined operation of parity, time-reversal, and signature symmetries ensures an absence of one of the signature partner band from the observed antimagnetic spectrum. This formalism has also been tested for the recently observed negative parity Δ I =2 antimagnetic spectrum in odd-A 101Pd nucleus and explains nicely its energy spectrum as well as the B (E 2 ) values. Further, this formalism is found to be fully consistent with twin-shears mechanism popularly known for such type of rotational bands. It also provides significant clue for extending these experiments in various mass regions spread over the nuclear chart.

Analysis of Hubble Space Telescope Observations of an Outburst of Comet 29P/Schwassmann-Wachmann 1

NASA Astrophysics Data System (ADS)

Schambeau, Charles Alfred; Fernandez, Yanga R.; Samarasinha, Nalin H.; Kundu, Arunav

2016-10-01

We present results of a continuing analysis on the spin state of the enigmatic Comet 29P/Schwassmann-Wachmann 1 (SW1). Previous works have reported possible constraints on the spin state including a non-principal axis state [1] or a rotation period of tens of days [2]. This diversity of published answers highlights the complexity of determining the spin state of an active comet nucleus. Previous work by our group using 3D Monte Carlo coma modeling of ground-based outburst observations from 2008 [3] has placed constraints on the spin period for a set of assumed spin-pole orientations. Due to the nature of the 2008 outburst morphology no constraints on the spin-pole orientation could be found.We present here an analysis of Hubble Space Telescope WFPC2 observations of SW1 shortly after a 1996 outburst [4] with which we have further constrained the spin state. The 0.046-arcsec/pixel scale (176 km/pixel at SW1) of the PC detector gives an order-of-magnitude improvement in spatial resolution over our ground-based observations. Two sets of observations from UT 1996 Mar. 11.3 and 12.1 show the ejected dust forming an asymmetric outflow contained on the sunward side of the coma. A projected outflow velocity of 0.15 ± 0.02 km/s was measured, similar to our measured value from the 2008 observations. Enhancements of the images were performed [5] to bring out subtle variations in coma brightness (i.e., jets) and to allow us to search for signatures of the nucleus' rotation during the outburst. Three curved features are seen in both sets of observations and were modeled using the 3D Monte Carlo coma model [6]. We find a spin period on the order of several days, in agreement with our earlier 2008 analysis.[1] Meech, K. J., et al.: 1993, Astron. J., 106, 1222. [2] Miles, R., et al.: 2016, Icarus, 272, 327. [3] Schambeau, C. A., et al.: 2016, Icarus, submitted. [4] Feldman, P. D., et al.: 1996, AAS/DPS Meeting Abstracts, 28, 1084. [5] Samarasinha, N. and Larson, S.: 2014, Icarus, 239, 168. [6] Samarasinha, N. H., 2000, Astron. J. Letters, 529, L107-L110. We thank the Space Telescope Science Institute (AR14294), and the Center for Lunar and Asteroid Surface Science (CLASS, NNA14AB05A) for support of this work.

CONCERNING THE PROBLEM OF THE SYSTEMATIZATION OF $beta$ SPECTRA

DOE Office of Scientific and Technical Information (OSTI.GOV)

Seidl, R.

1956-01-01

S>From data on the energy liberated during KB capture or ing BETA decay, the problem of the construction of a shell model of the nucleus is considered. It is proposed at the BETA transition is carried out by the last particle in the shell. The neutron and proton levels are considered individually. It is stated, that on the basis of the data on topes and the values of the nuclear spins. To obtain agreement with the nuclear binding energies and the data on nuclear reactions, it becomes necessary to propose that the transition of each nucleon causes a lowering ofmore » the bottom of the potentisl well of the nucleus.« less

Control of electron spin decoherence in nuclear spin baths

NASA Astrophysics Data System (ADS)

Liu, Ren-Bao

2011-03-01

Nuclear spin baths are a main mechanism of decoherence of spin qubits in solid-state systems, such as quantum dots and nitrogen-vacancy (NV) centers of diamond. The decoherence results from entanglement between the electron and nuclear spins, established by quantum evolution of the bath conditioned on the electron spin state. When the electron spin is flipped, the conditional bath evolution is manipulated. Such manipulation of bath through control of the electron spin not only leads to preservation of the center spin coherence but also demonstrates quantum nature of the bath. In an NV center system, the electron spin effectively interacts with hundreds of 13 C nuclear spins. Under repeated flip control (dynamical decoupling), the electron spin coherence can be preserved for a long time (> 1 ms) . Thereforesomecharacteristicoscillations , duetocouplingtoabonded 13 C nuclear spin pair (a dimer), are imprinted on the electron spin coherence profile, which are very sensitive to the position and orientation of the dimer. With such finger-print oscillations, a dimer can be uniquely identified. Thus, we propose magnetometry with single-nucleus sensitivity and atomic resolution, using NV center spin coherence to identify single molecules. Through the center spin coherence, we could also explore the many-body physics in an interacting spin bath. The information of elementary excitations and many-body correlations can be extracted from the center spin coherence under many-pulse dynamical decoupling control. Another application of the preserved spin coherence is identifying quantumness of a spin bath through the back-action of the electron spin to the bath. We show that the multiple transition of an NV center in a nuclear spin bath can have longer coherence time than the single transition does, when the classical noises due to inhomogeneous broadening is removed by spin echo. This counter-intuitive result unambiguously demonstrates the quantumness of the nuclear spin bath. This work was supported by Hong Kong RGC/GRF CUHK402207, CUHK402209, and CUHK402410. The author acknowledges collaboration with Nan Zhao, Jian-Liang Hu, Sai Wah Ho, Jones T. K. Wan, and Jiangfeng Du.

Mass-energy distribution of fragments within Langevin dynamics of fission induced by heavy ions

NASA Astrophysics Data System (ADS)

Anischenko, Yu. A.; Adeev, G. D.

2012-08-01

A stochastic approach based on four-dimensional Langevin fission dynamics is applied to calculating mass-energy distributions of fragments originating from the fission of excited compound nuclei. In the model under investigation, the coordinate K representing the projection of the total angular momentum onto the symmetry axis of the nucleus is taken into account in addition to three collective shape coordinates introduced on the basis of the { c, h, α} parametrization. The evolution of the orientation degree of freedom ( K mode) is described by means of the Langevin equation in the overdamped regime. The tensor of friction is calculated under the assumption of the reducedmechanismof one-body dissipation in the wall-plus-window model. The calculations are performed for two values of the coefficient that takes into account the reduction of the contribution from the wall formula: k s = 0.25 and k s = 1.0. Calculations with a modified wall-plus-window formula are also performed, and the quantity measuring the degree to which the single-particle motion of nucleons within the nuclear system being considered is chaotic is used for k s in this calculation. Fusion-fission reactions leading to the production of compound nuclei are considered for values of the parameter Z 2/ A in the range between 21 and 44. So wide a range is chosen in order to perform a comparative analysis not only for heavy but also for light compound nuclei in the vicinity of the Businaro-Gallone point. For all of the reactions considered in the present study, the calculations performed within four-dimensional Langevin dynamics faithfully reproduce mass-energy and mass distributions obtained experimentally. The inclusion of the K mode in the Langevin equation leads to an increase in the variances of mass and energy distributions in relation to what one obtains from three-dimensional Langevin calculations. The results of the calculations where one associates k s with the measure of chaoticity in the single-particle motion of nucleons within the nuclear system under study are in good agreement for variances of mass distributions. The results of calculations for the correlations between the prescission neutron multiplicity and the fission-fragment mass, < n pre( M)>, and between, this multiplicity and the kinetic energy of fission fragments, < n pre( E k )>, are also presented.

High-seniority states in spherical nuclei: Triple pair breaking in tin isotopes

NASA Astrophysics Data System (ADS)

Astier, Alain

2013-03-01

The 119-126Sn nuclei have been produced as fission fragments in two reactions induced by heavy ions: 12C+238U at 90 MeV bombarding energy, 18O+208Pb at 85 MeV. Their level schemes have been built from gamma rays detected using the Euroball array. High-spin states located above the long-lived isomeric states of the even- A and odd-A 120-126Sn nuclei have been identified. Moreover isomeric states lying around 4.5 MeV have been established in the even-A 120-126Sn from the delayed coincidences between the fission fragment detector SAPhIR and the Euroball array. All the states located above 3-MeV excitation energy are ascribed to several broken pairs of neutrons occupying the h11/2 orbit. The maximum value of angular momentum available in such a high-j shell, i.e. for mid-occupation and the breaking of the three neutron pairs (seniority v=6), has been identified.

The resolved nucleus of Comet Siding Spring (C/2013 A1) in MRO HiRISE images

NASA Astrophysics Data System (ADS)

Farnham, Tony; Kelley, Michael S.; Bodewits, Dennis; Bauer, James M.

2017-10-01

Comet Siding Spring (C/2013 A1) passed within 140,000 km of Mars on 19 Oct 2014. The MRO spacecraft, in orbit around Mars, used its HiRISE camera to monitor the comet during the encounter, obtaining the first resolved images of the nucleus of a dynamically new comet.MRO observed Siding Spring from 60 hr before, to 15 hr after close approach, obtaining 122 images in three different color filters. Close approach images, with a spatial scale as small as 138 m/pix, reveal an elongated crescent that changes shape over the course of the sequence, indicating that we are seeing a ~1 km non-spherical body from different viewpoints as the comet rapidly sweeps past. To better constrain the characteristics of the nucleus, we are performing detailed analyses, including modeling of the inner coma to separate its flux contribution from that of the nucleus. In conjunction with the coma removal, we will model the nucleus as a prolate/triaxial ellipsoid and, combined with the known illumination and viewing conditions, will use the changing aspect in the images to constrain the size, shape, orientation, albedo and possibly the phase dependence of the nucleus.In addition to the close approach observations, the images before and after close approach capture the coma structure and brightness. The photometric lightcurve from these images shows variability with an 8.1 hr period, which is presumed to be the rotational modulation of the coma activity. The observed morphology changes as well, promising to provide a measure of the nucleus' spin axis orientation.We will report on the results from our analyses, and provide the first direct measurements of the nucleus of a dynamically new comet.

Fission dynamics with microscopic level densities

NASA Astrophysics Data System (ADS)

Randrup, Jørgen; Ward, Daniel; Carlsson, Gillis; Døssing, Thomas; Möller, Peter; Åberg, Sven

2018-03-01

Working within the Langevin framework of nuclear shape dynamics, we study the dependence of the evolution on the degree of excitation. As the excitation energy of the fissioning system is increased, the pairing correlations and the shell effects diminish and the effective potential-energy surface becomes ever more liquid-drop like. This feature can be included in the treatment in a formally well-founded manner by using the local level densities as a basis for the shape evolution. This is particularly easy to understand and implement in the Metropolis treatment where the evolution is simulated by means of a random walk on the five-dimensional lattice of shapes for which the potential energy has been tabulated. Because the individual steps between two neighboring lattice sites are decided on the basis of the ratio of the statistical weights, what is needed is the ratio of the local level densities for those shapes, evaluated at the associated local excitation energies. For this purpose, we adapt a recently developed combinatorial method for calculating level densities which employs the same single-particle levels as those that were used for the calculation of the pairing and shell contributions to the macroscopic-microscopic deformation-energy surface. For each nucleus under consideration, the level density (for a fixed total angular momentum) is calculated microscopically for each of the over five million shapes given in the three-quadratic-surface parametrization. This novel treatment, which introduces no new parameters, is illustrated for the fission fragment mass distributions for selected uranium and plutonium cases.

Spectroscopic criteria for identification of nuclear tetrahedral and octahedral symmetries: Illustration on a rare earth nucleus

NASA Astrophysics Data System (ADS)

Dudek, J.; Curien, D.; Dedes, I.; Mazurek, K.; Tagami, S.; Shimizu, Y. R.; Bhattacharjee, T.

2018-02-01

We formulate criteria for identification of the nuclear tetrahedral and octahedral symmetries and illustrate for the first time their possible realization in a rare earth nucleus 152Sm. We use realistic nuclear mean-field theory calculations with the phenomenological macroscopic-microscopic method, the Gogny-Hartree-Fock-Bogoliubov approach, and general point-group theory considerations to guide the experimental identification method as illustrated on published experimental data. Following group theory the examined symmetries imply the existence of exotic rotational bands on whose properties the spectroscopic identification criteria are based. These bands may contain simultaneously states of even and odd spins, of both parities and parity doublets at well-defined spins. In the exact-symmetry limit those bands involve no E 2 transitions. We show that coexistence of tetrahedral and octahedral deformations is essential when calculating the corresponding energy minima and surrounding barriers, and that it has a characteristic impact on the rotational bands. The symmetries in question imply the existence of long-lived shape isomers and, possibly, new waiting point nuclei—impacting the nucleosynthesis processes in astrophysics—and an existence of 16-fold degenerate particle-hole excitations. Specifically designed experiments which aim at strengthening the identification arguments are briefly discussed.

The LOCV asymmetric nuclear matter two-body density distributions versus those of FHNC

NASA Astrophysics Data System (ADS)

Tafrihi, Azar

2018-05-01

The theoretical computations of the electron-nucleus scattering can be improved, by employing the asymmetric nuclear matter (ASM) two-body density distributions (TBDD) . But, due to the sophistications of the calculations, the TBDD with arbitrary isospin asymmetry have not yet been computed in the Fermi Hypernetted Chain (FHNC) or the Monte Carlo (MC) approaches. So, in the present work, we intend to find the ASM TBDD, in the states with isospin T, spin S and spin projection Sz, in the Lowest Order Constrained Variational (LOCV) method. It is demonstrated that, at small relative distances, independent of the proton to neutron ratio β, the state-dependent TBDD have a universal shape. Expectedly, it is observed that, at low (high) β values, the nucleons prefer to make a pair in the T = 1(0) states. In addition, the strength of the tensor-dependent correlations is investigated, using the ratio of the TBDD in the TSSz = 010 state with θ = π / 2 and that of θ = 0. The mentioned ratios peak at r ∼ 0 . 9 fm, considering different β values. It is hoped that, the present results could help a better reproduction of the experimental data of the electron-nucleus scattering.

Nuclear Spin Dependent Parity Violation in Diatomic Molecules

NASA Astrophysics Data System (ADS)

Altuntas, Emine; Cahn, Sidney; Demille, David; Kozlov, Mikhail

2016-05-01

Nuclear spin-dependent parity violation (NSD-PV) effects arise from exchange of the Z0 boson between electrons and the nucleus, and from interaction of electrons with the nuclear anapole moment, a parity-odd magnetic moment. The latter scales with nucleon number of the nucleus A as A 2 / 3 , whereas the Z0 coupling is independent of A. Thus the former is the dominant source of NSD-PV for nuclei with A >= 20. We study NSD-PV effects using diatomic molecules, where signals are dramatically amplified by bringing rotational levels of opposite parity close to degeneracy in a strong magnetic field. The NSD-PV interaction matrix element is measured using a Stark-interference technique. We present results that demonstrate statistical sensitivity to NSD-PV effects surpassing that of any previous atomic parity violation measurement, using the test system 138 Ba19 F. We report our progress on measuring and cancelling systematic effects due to combination of non-reversing stray E-fields, Enr with B-field inhomogeneities. Short-term prospects for measuring the nuclear anapole moment of 137 Ba19 F are discussed. In the long term, our technique is sufficiently general and sensitive to enable measurements across a broad range of nuclei.

Nuclear Spin Dependent Parity Violation in Diatomic Molecules

NASA Astrophysics Data System (ADS)

Altuntas, Emine; Cahn, Sidney; Demille, David

2016-09-01

Nuclear spin-dependent parity violation (NSD-PV) effects arise from exchange of the Z0 boson between electrons and the nucleus, and from interaction of electrons with the nuclear anapole moment, a parity-odd magnetic moment. The latter scales with nucleon number of the nucleus A as A2/3 , whereas the Z0 coupling is independent of A. Thus the former is the dominant source of NSD-PV for nuclei with A >= 20 . We study NSD-PV effects using diatomic molecules, where signals are dramatically amplified by bringing rotational levels of opposite parity close to degeneracy in a strong magnetic field. The NSD-PV interaction matrix element is measured using a Stark-interference technique. We present results that demonstrate statistical sensitivity to NSD-PV effects surpassing that of any previous atomic parity violation measurement, using the test system 138Ba19F. We report our progress on measuring and cancelling systematic effects due to combination of non-reversing stray E-fields, Enr with B-field inhomogeneities. Short-term prospects for measuring the nuclear anapole moment of 137Ba19F are discussed. In the long term, our technique is sufficiently general and sensitive to enable measurements across a broad range of nuclei.

Nuclear Spin Dependent Parity Violation in Diatomic Molecules

NASA Astrophysics Data System (ADS)

Altuntas, Emine; Ammon, Jeffrey; Cahn, Sidney; Demille, David; Kozlov, Mikhail; Paolino, Richard

2015-05-01

Nuclear spin-dependent parity violation (NSD-PV) effects arise from exchange of the Z0 boson between electrons and the nucleus, and from interaction of electrons with the nuclear anapole moment, a parity-odd magnetic moment. The latter scales with nucleon number of the nucleus A as A 2 / 3 , whereas the Z0 coupling is independent of A. Thus the former is the dominant source of NSD-PV for nuclei with A >= 20. We study NSD-PV effects using diatomic molecules, where signals are dramatically amplified by bringing rotational levels of opposite parity close to degeneracy in a strong magnetic field. Using a Stark-interference technique we measure the NSD-PV interaction matrix element. We present results that demonstrate statistical sensitivity to NSD-PV effects surpassing that of any previous atomic parity violation measurement, using the test system 138Ba19F. We also discuss investigations of systematics due to non-reversing stray E-fields, Enr together with B-field inhomogeneities, and short-term prospects for measuring the nuclear anapole moment of 137Ba. In the long term, our technique is sufficiently general and sensitive to enable measurements across a broad range of nuclei.

First Exclusive Measurement of Deeply Virtual Compton Scattering off He 4 : Toward the 3D Tomography of Nuclei

DOE PAGES

Hattawy, M.; Baltzell, N. A.; Dupré, R.; ...

2017-11-15

Here, we report on the first measurement of the beam-spin asymmetry in the exclusive process of coherent deeply virtual Compton scattering off a nucleus. The experiment used the 6 GeV electron beam from the CEBAF accelerator at Jefferson Lab incident on a pressurizedmore » $^4$He gaseous target placed in front of the CEBAF Large Acceptance Spectrometer (CLAS). The scattered electron was detected by CLAS and the photon by a dedicated electromagnetic calorimeter at forward angles. To ensure the exclusivity of the process, a specially designed radial time projection chamber was used to detect the recoiling $^4$He nuclei. We measured beam-spin asymmetries larger than those observed on the free proton in the same kinematic domain. From these, we were able to extract, in a model-independent way, the real and imaginary parts of the only $^4$He Compton form factor, $$\\cal H_A$$. This first measurement of coherent deeply virtual Compton scattering on the $^4$He nucleus, with a fully exclusive final state via nuclear recoil tagging, leads the way toward 3D imaging of the partonic structure of nuclei.« less

Study on reaction mechanism by analysis of kinetic energy spectra of light particles and formation of final products

NASA Astrophysics Data System (ADS)

Giardina, G.; Mandaglio, G.; Nasirov, A. K.; Anastasi, A.; Curciarello, F.; Fazio, G.

2018-05-01

The sensitivity of reaction mechanism in the formation of compound nucleus (CN) by the analysis of kinetic energy spectra of light particles and of reaction products are shown. The dependence of the P CN fusion probability of reactants and W sur survival probability of CN against fission at its deexcitation on the mass and charge symmetries in the entrance channel of heavy-ion collisions, as well as on the neutron numbers is discussed. The possibility of conducting a complex program of investigations of the complete fusion by reliable ways depends on the detailed and refined methods of experimental and theoretical analyses.

Quantifying the quantum gate fidelity of single-atom spin qubits in silicon by randomized benchmarking.

PubMed

Muhonen, J T; Laucht, A; Simmons, S; Dehollain, J P; Kalra, R; Hudson, F E; Freer, S; Itoh, K M; Jamieson, D N; McCallum, J C; Dzurak, A S; Morello, A

2015-04-22

Building upon the demonstration of coherent control and single-shot readout of the electron and nuclear spins of individual (31)P atoms in silicon, we present here a systematic experimental estimate of quantum gate fidelities using randomized benchmarking of 1-qubit gates in the Clifford group. We apply this analysis to the electron and the ionized (31)P nucleus of a single P donor in isotopically purified (28)Si. We find average gate fidelities of 99.95% for the electron and 99.99% for the nuclear spin. These values are above certain error correction thresholds and demonstrate the potential of donor-based quantum computing in silicon. By studying the influence of the shape and power of the control pulses, we find evidence that the present limitation to the gate fidelity is mostly related to the external hardware and not the intrinsic behaviour of the qubit.

Exploring methods to expedite the recording of CEST datasets using selective pulse excitation

NASA Astrophysics Data System (ADS)

Yuwen, Tairan; Bouvignies, Guillaume; Kay, Lewis E.

2018-07-01

Chemical Exchange Saturation Transfer (CEST) has emerged as a powerful tool for studies of biomolecular conformational exchange involving the interconversion between a major, visible conformer and one or more minor, invisible states. Applications typically entail recording a large number of 2D datasets, each of which differs in the position of a weak radio frequency field, so as to generate a CEST profile for each nucleus from which the chemical shifts of spins in the invisible state(s) are obtained. Here we compare a number of band-selective CEST schemes for speeding up the process using either DANTE or cosine-modulated excitation approaches. We show that while both are essentially identical for applications such as 15N CEST, in cases where the probed spins are dipolar or scalar coupled to other like spins there can be advantages for the cosine-excitation scheme.

High spin structure and intruder configurations in 31P

NASA Astrophysics Data System (ADS)

Ionescu-Bujor, M.; Iordachescu, A.; Napoli, D. R.; Lenzi, S. M.; Mărginean, N.; Otsuka, T.; Utsuno, Y.; Ribas, R. V.; Axiotis, M.; Bazzacco, D.; Bizzeti-Sona, A. M.; Bizzeti, P. G.; Brandolini, F.; Bucurescu, D.; Cardona, M. A.; De Angelis, G.; De Poli, M.; Della Vedova, F.; Farnea, E.; Gadea, A.; Hojman, D.; Kalfas, C. A.; Kröll, Th.; Lunardi, S.; Martínez, T.; Mason, P.; Pavan, P.; Quintana, B.; Alvarez, C. Rossi; Ur, C. A.; Vlastou, R.; Zilio, S.

2006-02-01

The nucleus 31P has been studied in the 24Mg(16O,2αp) reaction with a 70-MeV 16O beam. A complex level scheme extended up to spins 17/2+ and 15/2-, on positive and negative parity, respectively, has been established. Lifetimes for the new states have been investigated by the Doppler shift attenuation method. Two shell-model calculations have been performed to describe the experimental data, one by using the code ANTOINE in a valence space restricted to the sd shell, and the other by applying the Monte Carlo shell model in a valence space including the sd-fp shells. The latter calculation indicates that intruder excitations, involving the promotion of a T=0 proton-neutron pair to the fp shell, play a dominant role in the structure of the positive-parity high-spin states of 31P.

New Global Calculation of Nuclear Masses and Fission Barriers for Astrophysical Applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Moeller, P.; Sierk, A. J.; Bengtsson, R.

The FRDM(1992) mass model [1] has an accuracy of 0.669 MeV in the region where its parameters were determined. For the 529 masses that have been measured since, its accuracy is 0.46 MeV, which is encouraging for applications far from stability in astrophysics. We are developing an improved mass model, the FRDM(2008). The improvements in the calculations with respect to the FRDM(1992) are in two main areas. (1) The macroscopic model parameters are better optimized. By simulation (adjusting to a limited set of now known nuclei) we can show that this actually makes the results more reliable in new regionsmore » of nuclei. (2) The ground-state deformation parameters are more accurately calculated. We minimize the energy in a four-dimensional deformation space ({epsilon}{sub 2}, {epsilon}{sub 3}, {epsilon}{sub 4}, {epsilon}{sub 6},) using a grid interval of 0.01 in all 4 deformation variables. The (non-finalized) FRDM (2008-a) has an accuracy of 0.596 MeV with respect to the 2003 Audi mass evaluation before triaxial shape degrees of freedom are included (in progress). When triaxiality effects are incorporated preliminary results indicate that the model accuracy will improve further, to about 0.586 MeV.We also discuss very large-scale fission-barrier calculations in the related FRLDM (2002) model, which has been shown to reproduce very satisfactorily known fission properties, for example barrier heights from {sup 70}Se to the heaviest elements, multiple fission modes in the Ra region, asymmetry of mass division in fission and the triple-humped structure found in light actinides. In the superheavy region we find barriers consistent with the observed half-lives. We have completed production calculations and obtain barrier heights for 5254 nuclei heavier than A = 170 for all nuclei between the proton and neutron drip lines. The energy is calculated for 5009325 different shapes for each nucleus and the optimum barrier between ground state and separated fragments is determined by use of an ''immersion'' technique.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Younes, W; Britt, H C; Wilhelmy, J B

The purpose of this note is to combine existing information on the {sup 237}U(n,f) cross section to determine if some consistency can be obtained for the neutron induced fission excitation of {sup 237}U. The neutron induced fission cross section of the 6.8 day {sup 237}U was measured directly by McNally et al. in 1968 using the Pommard nuclear device test. At the same time critical assembly measurements were done at Los Alamos using the Flattop assembly. A previous measurement was also made at LASL in 1954 with two different neutron sources, each peaked near 200 keV. The results were 0.66more » {+-} 0.10 b and 0.70 {+-} 0.07 b for the (n,f) cross section. More recently Younes and Britt have reanalyzed direct reaction charged particle data of Cramer and Britt that had determined the fission probability of the {sup 238}U compound nucleus as a function of nuclear excitation energy. They have combined fission probabilities with calculated neutron absorption cross sections, including corrections for the differences in angular momentum between the direct and neutron induced reactions. From this analysis they have extracted equivalent {sup 237}U(n,f) cross sections. The technique for extracting surrogate (n,f) cross sections from (t,pf) data has been demonstrated in a recent publication for the test case {sup 235}U(n,f). In addition to this experimental information, Lynn and Hayes have recently done a new theoretical study of the fission cross sections for a series of isotopes in this region. A summary plot of the data is shown in Fig. 1. Below 0.5 MeV the McNally, Cowan, and Younes-Britt results are in reasonable agreement. The average cross section in the Younes-Britt results, for En = 0.1 to 0.4 MeV, is 0.80 times the McNally values which is well within the errors of the McNally experiment. Above 0.5 MeV the McNally results diverge toward higher values. It should be noted that this divergence begins approximately at the {sup 237}Np threshold and that {sup 237}Np is the daughter of the 6.8 day {sup 237}U decay.« less

WILL COMET ISON (C/2012 S1) SURVIVE PERIHELION?

DOE Office of Scientific and Technical Information (OSTI.GOV)

Knight, Matthew M.; Walsh, Kevin J., E-mail: knight@lowell.edu

2013-10-10

On 2013 November 28 Comet ISON (C/2012 S1) will pass by the Sun with a perihelion distance of 2.7 solar radii. Understanding the possible outcomes for the comet's response to such a close passage by the Sun is important for planning observational campaigns and for inferring ISON's physical properties. We present new numerical simulations and interpret them in context with the historical track record of comet disruptions and of sungrazing comet behavior. Historical data suggest that sizes below ∼200 m are susceptible to destruction by sublimation driven mass loss, while we find that for ISON's perihelion distance, densities lower thanmore » 0.1 g cm{sup –3} are required to tidally disrupt a retrograde or non-spinning body. Such low densities are substantially below the range of the best-determined comet nucleus densities, though dynamically new comets such as ISON have few measurements of physical properties. Disruption may occur for prograde rotation at densities up to 0.7 g cm{sup –3}, with the chances of disruption increasing for lower density, faster prograde rotation, and increasing elongation of the nucleus. Given current constraints on ISON's nucleus properties and the typically determined values for these properties among all comets, we find tidal disruption to be unlikely unless other factors (e.g., spin-up via torquing) affect ISON substantially. Whether or not disruption occurs, the largest remnant must be big enough to survive subsequent mass loss due to sublimation in order for ISON to remain a viable comet well after perihelion.« less

High-spin structures in the 139Pr nucleus

NASA Astrophysics Data System (ADS)

Yeoh, E. Y.; Zhu, S. J.; Wang, J. G.; Xiao, Z. G.; Zhang, M.; Yan, W. H.; Wang, R. S.; Xu, Q.; Wu, X. G.; He, C. Y.; Li, G. S.; Zheng, Y.; Li, C. B.; Cao, X. P.; Hu, S. P.; Yao, S. H.; Yu, B. B.

2012-06-01

Background: 139Pr is located in a transitional region of neutron number close to the N=82 shell. The study of its high-spin states and collective bands is important for systematically understanding the nuclear structural characteristics in this region.Purpose: To investigate the high-spin levels and to search for oblate bands in 139Pr.Methods: The high-spin states of 139Pr have been studied via the reaction 124Sn(19F,4n) at a beam energy of 80 MeV. The experiment was carried out at the HI-13 Tandem Accelerator at the China Institute of Atomic Energy (CIAE). The data analysis was done by using the γ-γ coincidence method.Results: The level scheme of 139Pr has been expanded with spin up to 45/2ℏ. A total of 39 new levels and 45 new transitions are identified. Four collective band structures at high-spin states have been newly established. From systematic analysis, one of the bands is proposed as a double decoupled band; two bands are proposed as oblate bands with γ˜-60∘; another band is suggested as an oblate-triaxial band with γ˜-90∘. The other characteristics for these bands are discussed.Conclusions: A new level scheme in 139Pr has been established and the collective bands at high spin have been identified. The result shows that the strong oblate shape-driving effect is caused by neutrons at the high-spin states in 139Pr.

Angstrom-Resolution Magnetic Resonance Imaging of Single Molecules via Wave-Function Fingerprints of Nuclear Spins

NASA Astrophysics Data System (ADS)

Ma, Wen-Long; Liu, Ren-Bao

2016-08-01

Single-molecule sensitivity of nuclear magnetic resonance (NMR) and angstrom resolution of magnetic resonance imaging (MRI) are the highest challenges in magnetic microscopy. Recent development in dynamical-decoupling- (DD) enhanced diamond quantum sensing has enabled single-nucleus NMR and nanoscale NMR. Similar to conventional NMR and MRI, current DD-based quantum sensing utilizes the "frequency fingerprints" of target nuclear spins. The frequency fingerprints by their nature cannot resolve different nuclear spins that have the same noise frequency or differentiate different types of correlations in nuclear-spin clusters, which limit the resolution of single-molecule MRI. Here we show that this limitation can be overcome by using "wave-function fingerprints" of target nuclear spins, which is much more sensitive than the frequency fingerprints to the weak hyperfine interaction between the targets and a sensor under resonant DD control. We demonstrate a scheme of angstrom-resolution MRI that is capable of counting and individually localizing single nuclear spins of the same frequency and characterizing the correlations in nuclear-spin clusters. A nitrogen-vacancy-center spin sensor near a diamond surface, provided that the coherence time is improved by surface engineering in the near future, may be employed to determine with angstrom resolution the positions and conformation of single molecules that are isotope labeled. The scheme in this work offers an approach to breaking the resolution limit set by the "frequency gradients" in conventional MRI and to reaching the angstrom-scale resolution.

Results from the First {sup 249}Cf + {sup 48}Ca Experiment

DOE R&D Accomplishments Database

Oganessian, Y. T.; Utyonkov, V. K.; Lobanov, Y. V.; Abdullin, F. S.; Polyakov, A. N.; Shirokovsky, I. V.; Tsyganov, Y. S.; Mezentsev, A. N.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Ivanov, O. V.; Voinov, A. A.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Moody, K. J.; Wild, J. F.; Stoyer, M. A.; Stoyer, N. J.; Laue, C. A.; Shaughnessy, D. A.; Patin, J. B.; Lougheed, R. W.

2003-02-03

The present paper reports the results of an attempt aimed at the synthesis of element 118 in the reaction {sup 249}Cf({sup 48}Ca,3n){sup 294}118. The experiment was performed employing the Dubna Gas-filled Recoil Separator and the U400 heavy-ion cyclotron at FLNR, JINR, Dubna. In the course of a 2300-hour irradiation of an enriched {sup 249}Cf target (0.23 mg/cm{sup 2}) with a beam of 245-MeV {sup 48}Ca ions, we accumulated a total beam dose of 2.5 x 10{sup 19} ions. We detected two events that may be attributed to the formation and decay of nuclei with Z=118. For one event, we observed a decay chain of two correlated {alpha}-decays with corresponding energies and correlation times of E{sub {alpha}1} = 11.65 {+-} 0.06 MeV, t{sub {alpha}1} = 2.55 ms and E{sub {alpha}2} = 10.71 {+-} 0.17 MeV, t{sub {alpha}2} = 42.1 ms and, finally, a spontaneous fission with the sum of the kinetic energies of the fission fragments E{sub tot} = 207 MeV (TKE {approx} 230 MeV) and t{sub SF} = 0.52 s. In the second event chain, the recoil nucleus decayed into two fission fragments with E{sub tot} = 223 MeV (TKE {approx} 245 MeV) 3.16 ms later, without intervening {alpha} decays. The probabilities that these events were caused by the chance correlations of unrelated signals are negligible. Both events were observed at an excitation energy of the compound nucleus {sup 297}118 of E* = 30.0 {+-} 2.4 MeV, close to the expected maximum of the 3n-evaporation channel. The relationship between the decay energy Q{sub {alpha}} and decay period T{sub {alpha}} shows that sequential {alpha}-transitions in the first event correspond to the decay chain with Z = 118{_}116{_}114. Decay characteristics of the newly observed nuclides are compared with radioactive decay properties of the even-even isotopes with Z = 116, 114 and 112 previously produced in the reactions {sup 244}Pu, {sup 248}Cm + {sup 48}Ca and calculations made in various nuclear models.

Relativistic Corrections to the Energy of the Electron in a Hydrogenlike Atom

NASA Astrophysics Data System (ADS)

Skobelev, V. V.

2017-11-01

Using the previously found solution of the Dirac equation for an electron in the field of the nucleus ( Ze), expressed in terms of the eigenfunction of the spin projection operator Σ3, in the expansion in the small parameter ( Zα), α = e 2/ ħc ≈ 1/137, relativistic and spin-orbit corrections to the energy of the electron in a hydrogenlike atom are calculated, where the latter, in our view, are represented in an easier to visualize form in comparison with previously known classical results. This work may be of methodological interest in the sense of some modification of the corresponding sections of the traditional course on quantum mechanics.

Spin-locking of half-integer quadrupolar nuclei in nuclear magnetic resonance of solids: second-order quadrupolar and resonance offset effects.

PubMed

Ashbrook, Sharon E; Wimperis, Stephen

2009-11-21

Spin-locking of spin I=3/2 and I=5/2 nuclei in the presence of small resonance offset and second-order quadrupolar interactions has been investigated using both exact and approximate theoretical and experimental nuclear magnetic resonance (NMR) approaches. In the presence of second-order quadrupolar interactions, we show that the initial rapid dephasing that arises from the noncommutation of the state prepared by the first pulse and the spin-locking Hamiltonian gives rise to tensor components of the spin density matrix that are antisymmetric with respect to inversion, in addition to those symmetric with respect to inversion that are found when only a first-order quadrupolar interaction is considered. We also find that spin-locking of multiple-quantum coherence in a static solid is much more sensitive to resonance offset than that of single-quantum coherence and show that good spin-locking of multiple-quantum coherence can still be achieved if the resonance offset matches the second-order shift of the multiple-quantum coherence in the appropriate reference frame. Under magic angle spinning (MAS) conditions, and in the "adiabatic" limit, we demonstrate that rotor-driven interconversion of central-transition single- and three-quantum coherences for a spin I=3/2 nucleus can be best achieved by performing the spin-locking on resonance with the three-quantum coherence in the three-quantum frame. Finally, in the "sudden" MAS limit, we show that spin I=3/2 spin-locking behavior is generally similar to that found in static solids, except when the central-transition nutation rate matches a multiple of the MAS rate and a variety of rotary resonance phenomena are observed depending on the internal spin interactions present. This investigation should aid in the application of spin-locking techniques to multiple-quantum NMR of quadrupolar nuclei and of cross-polarization and homonuclear dipolar recoupling experiments to quadrupolar nuclei such as (7)Li, (11)B, (17)O, (23)Na, and (27)Al.

Dark sequential Z ' portal: Collider and direct detection experiments

NASA Astrophysics Data System (ADS)

Arcadi, Giorgio; Campos, Miguel D.; Lindner, Manfred; Masiero, Antonio; Queiroz, Farinaldo S.

2018-02-01

We revisit the status of a Majorana fermion as a dark matter candidate when a sequential Z' gauge boson dictates the dark matter phenomenology. Direct dark matter detection signatures rise from dark matter-nucleus scatterings at bubble chamber and liquid xenon detectors, and from the flux of neutrinos from the Sun measured by the IceCube experiment, which is governed by the spin-dependent dark matter-nucleus scattering. On the collider side, LHC searches for dilepton and monojet + missing energy signals play an important role. The relic density and perturbativity requirements are also addressed. By exploiting the dark matter complementarity we outline the region of parameter space where one can successfully have a Majorana dark matter particle in light of current and planned experimental sensitivities.

Polarization effects in the reactions p + 3 He → π+ + 4 He, π+ + 4 He → p + 3 He and quantum character of spin correlations in the final (p, 3 He) system

NASA Astrophysics Data System (ADS)

Lyuboshitz, Valery V.; Lyuboshitz, Vladimir L.

2017-12-01

The general consequences of T invariance for the direct and inverse binary reactions a + b → c + d, c + d → a + b with spin-1/2 particles a, b and unpolarized particles c, d are considered. Using the formalism of helicity amplitudes, the polarization effects are studied in the reaction p + 3 He → π+ + 4 He and in the inverse process π+ + 4 He → p + 3 He. It is shown that in the reaction π + + 4 He → p + 3 He the spins of the final proton and 3 He nucleus are strongly correlated. A structural expression through helicity amplitudes, corresponding to arbitrary emission angles, is obtained for the correlation tensor. It is established that in the reaction π + + 4 He → p + 3 He one of the “classical” incoherence inequalities of the Bell type for diagonal components of the correlation tensor is necessarily violated and, thus, the spin correlations of the final particles have the strongly pronounced quantum character.

High spin states of 141Pm

NASA Astrophysics Data System (ADS)

Bhattacharyya, Sarmishtha; Chanda, Somen; Bhattacharjee, Tumpa; Basu, Swapan Kumar; Bhowmik, R. K.; Muralithar, S.; Singh, R. P.; Ghugre, S. S.

2004-01-01

The high spin states in the N=80 odd- A141Pm nucleus have been investigated by in-beam γ-spectroscopic techniques following the reaction 133Cs( 12C, 4n) 141Pm at E=65 MeV using a modest γ detector array, consisting of seven Compton-suppressed high purity germanium detectors and a multiplicity ball of 14 bismuth germanate elements. Thirty new γ rays have been assigned to 141Pm on the basis of γ-ray singles and γγ-coincidence data. The level scheme of 141Pm has been extended upto an excitation energy of 5.2 MeV and spin {35}/{2}ℏ and 16 new levels have been proposed. Spin-parity assignments for most of the newly proposed levels have been made on the basis of the deduced directional correlation orientation ratios for strong transitions. The meanlives of a few excited states have been determined from the pulsed beam- γγ coincidence data using the generalised centroid-shift method. The level structure is discussed in the light of known systematics of neighbouring N=80 isotonic nuclei.

Prompt photon measurements with PHENIX's MPC-EX detector

NASA Astrophysics Data System (ADS)

Campbell, Sarah; PHENIX Collaboration

2013-08-01

The MPC-EX detector is a Si-W preshower extension to the existing Muon Piston Calorimeter (MPC). The MPC-EX consists of eight layers of alternating W absorber and Si mini-pad sensors. Located at forward rapidity, 3.1 < |η| < 3.8, the MPC and MPC-EX will access low-x partons in the Au nucleus in p+Au collisions and high-x partons in the projectile in polarized p+p collisions. With the addition of the MPC-EX, the neutral pion reconstruction energy range extends to the luminosity limit, energies > 80 GeV, a factor of four improvement over current capabilities. Not only will the MPC-EX strengthen PHENIX's existing forward π0 and jet measurements, it will provide sufficient prompt photon and π0 separation to make a prompt photon measurement possible. Prompt photon yields at high pT, pT > 3 GeV/c, can be statistically extracted using the double ratio method. In transversely polarized p+p collisions, the measurement of the prompt photon single spin asymmetry, AN, will resolve the sign discrepancy between the Sivers and twist-3 extractions of AN. In p+Au collisions, the prompt photon RpAu will quantify the level of gluon saturation in the Au nucleus at low-x, x ~ 10-3, with a projected systematic error band a factor of four smaller than EPS09's current allowable range. The MPC-EX detector will expand our understanding of the gluon nuclear parton distribution functions, providing important information about the initial state of heavy ion collisions, and clarify how the valence parton's transverse momentum and spin correlates to the proton spin.

Weakly interacting massive particle-nucleus elastic scattering response

NASA Astrophysics Data System (ADS)

Anand, Nikhil; Fitzpatrick, A. Liam; Haxton, W. C.

2014-06-01

Background: A model-independent formulation of weakly interacting massive particle (WIMP)-nucleon scattering was recently developed in Galilean-invariant effective field theory. Purpose: Here we complete the embedding of this effective interaction in the nucleus, constructing the most general elastic nuclear cross section as a factorized product of WIMP and nuclear response functions. This form explicitly defines what can and cannot be learned about the low-energy constants of the effective theory—and consequently about candidate ultraviolet theories of dark matter—from elastic scattering experiments. Results: We identify those interactions that cannot be reliably treated in a spin-independent/spin-dependent (SI/SD) formulation: For derivative- or velocity-dependent couplings, the SI/SD formulation generally mischaracterizes the relevant nuclear operator and its multipolarity (e.g., scalar or vector) and greatly underestimates experimental sensitivities. This can lead to apparent conflicts between experiments when, in fact, none may exist. The new nuclear responses appearing in the factorized cross section are related to familiar electroweak nuclear operators such as angular momentum l⃗(i) and the spin-orbit coupling σ⃗(i).l⃗(i). Conclusions: To unambiguously interpret experiments and to extract all of the available information on the particle physics of dark matter, experimentalists will need to (1) do a sufficient number of experiments with nuclear targets having the requisite sensitivities to the various operators and (2) analyze the results in a formalism that does not arbitrarily limit the candidate operators. In an appendix we describe a code that is available to help interested readers implement such an analysis.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ryabov, E.G.; Adeev, G.D.

A macroscopic temperature-dependent model that takes into account nuclear forces of finite range is used to calculate the static and statistical properties of hot rotating compound nuclei. The level-density parameter is approximated by an expression of the leptodermous type. The resulting expansion coefficients are in good agreement with their counterparts proposed previously by A.V. Ignatyuk and his colleagues. The effect of taking simultaneously into account the temperature of a nucleus and its angular momentum on the quantities under study, such as the heights and positions of fission barriers and the effective moments of inertia of nuclei at the barrier, ismore » considered, and the importance of doing this is demonstrated. The fissility parameter (Z{sup 2}/A){sub crit} and the position of the Businaro-Gallone point are studied versus temperature. It is found that, with increasing temperature, both parameters are shifted to the region of lighter nuclei. It is shown that the inclusion of temperature leads to qualitatively the same effects as the inclusion of the angular momentum of a nucleus, but, quantitatively, thermal excitation leads to smaller effects than rotational excitation.« less

Experiment and Theory for Nuclear Reactions in Nano-Materials Show e14 - e16 Solid-State Fusion Reactions

NASA Astrophysics Data System (ADS)

George, Russ

2005-03-01

Nano-lattices of deuterium loving metals exhibit coherent behavior by populations of deuterons (d's) occupying a Bloch state. Therein, coherent d-overlap occurs wherein the Bloch condition reduces the Coulomb barrier.Overlap of dd pairs provides a high probability fusion will/must occur. SEM photo evidence showing fusion events is now revealed by laboratories that load or flux d into metal nano-domains. Solid-state dd fusion creates an excited ^4He nucleus entangled in the large coherent population of d's.This contrasts with plasma dd fusion in collision space where an isolated excited ^4He nucleus seeks the ground state via fast particle emission. In momentum limited solid state fusion,fast particle emission is effectively forbidden.Photographed nano-explosive events are beyond the scope of chemistry. Corroboration of the nuclear nature derives from photographic observation of similar events on spontaneous fission, e.g. Cf. We present predictive theory, heat production, and helium isotope data showing reproducible e14 to e16 solid-state fusion reactions.

Search for long lived heaviest nuclei beyond the valley of stability

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chowdhury, P. Roy; Samanta, C.; Physics Department, Virginia Commonwealth University, Richmond, Virginia 23284-2000

2008-04-15

The existence of long lived superheavy nuclei (SHN) is controlled mainly by spontaneous fission and {alpha}-decay processes. According to microscopic nuclear theory, spherical shell effects at Z=114, 120, 126 and N=184 provide the extra stability to such SHN to have long enough lifetime to be observed. To investigate whether the so-called 'stability island' could really exist around the above Z, N values, the {alpha}-decay half-lives along with the spontaneous fission and {beta}-decay half-lives of such nuclei are studied. The {alpha}-decay half-lives of SHN with Z=102-120 are calculated in a quantum tunneling model with DDM3Y effective nuclear interaction using Q{sub {alpha}}more » values from three different mass formulas prescribed by Koura-Uno-Tachibana-Yamada (KUTY), Myers-Swiatecki (MS), and Muntian-Hofmann-Patyk-Sobiczewski (MMM). Calculation of spontaneous fission (SF) half-lives for the same SHN are carried out using a phenomenological formula and compared with SF half-lives predicted by Smolanczuk et al. A possible source of discrepancy between the calculated {alpha}-decay half-lives of some nuclei and the experimental data of GSI, JINR-FLNR, RIKEN, is discussed. In the region of Z=106-108 with N{approx}160-164, the {beta}-stable SHN {sub 106}{sup 268}Sg{sub 162} is predicted to have highest {alpha}-decay half-life (T{sub {alpha}}{approx}3.2 h) using Q{sub {alpha}} value from MMM. Interestingly, it is much greater than the recently measured T{sub {alpha}} ({approx}22 s) of deformed doubly magic {sub 108}{sup 270}Hs{sub 162} nucleus. A few fission-survived long-lived SHN which are either {beta}-stable or having large {beta}-decay half-lives are predicted to exist near {sup 294}110{sub 184}, {sup 293}110{sub 183}, {sup 296}112{sub 184}, and {sup 298}114{sub 184}. These nuclei might decay predominantly through {alpha}-particle emission.« less

The Hsk1(Cdc7) Replication Kinase Regulates Origin Efficiency

PubMed Central

Patel, Prasanta K.; Kommajosyula, Naveen; Rosebrock, Adam; Bensimon, Aaron; Leatherwood, Janet; Bechhoefer, John

2008-01-01

Origins of DNA replication are generally inefficient, with most firing in fewer than half of cell cycles. However, neither the mechanism nor the importance of the regulation of origin efficiency is clear. In fission yeast, origin firing is stochastic, leading us to hypothesize that origin inefficiency and stochasticity are the result of a diffusible, rate-limiting activator. We show that the Hsk1-Dfp1 replication kinase (the fission yeast Cdc7-Dbf4 homologue) plays such a role. Increasing or decreasing Hsk1-Dfp1 levels correspondingly increases or decreases origin efficiency. Furthermore, tethering Hsk1-Dfp1 near an origin increases the efficiency of that origin, suggesting that the effective local concentration of Hsk1-Dfp1 regulates origin firing. Using photobleaching, we show that Hsk1-Dfp1 is freely diffusible in the nucleus. These results support a model in which the accessibility of replication origins to Hsk1-Dfp1 regulates origin efficiency and provides a potential mechanistic link between chromatin structure and replication timing. By manipulating Hsk1-Dfp1 levels, we show that increasing or decreasing origin firing rates leads to an increase in genomic instability, demonstrating the biological importance of appropriate origin efficiency. PMID:18799612

Maruhn-Greiner Maximum for Confirmation of Low Energy Nuclear Reactions (LENR) via a Compound Nucleus with Double Magic Numbers

NASA Astrophysics Data System (ADS)

Hora, Heinrich; Miley, George

2007-03-01

One of the most convincing facts about LENR due to deuterons (ds) or protons of very high concentration in host metals of palladium is the measurement of the large scale minimum in the reaction probability with product elements centered around the nucleon number A = 153. The local maximum was measured in this region is similar to fission of uranium at A = 119 where the local maximum follows the Maruhn-Greiner mechanism^1. We suggest this phenomenon can be explained by the strong screening of the Maxwellian ds on the degenerate rigid electron background within the swimming electrons at the metal surface or thin filem interfaces. The deuterons behave like neutrals at distances of above 2 picometers (pm) and form clusters due to soft attraction in the range of thermal energy; 10 pm diameter clusters can react over long time scales (10^6 s) with Pd leading to double magic number compound nuclei 306x126 decaying via fission to an A=153 element distribution. J. Maruhn et al, Phys. Rev. Letters 32, 548 (1974) H. Hora, G.H. Miley, CzechJ. Phys. 48, 1111 (1998)

The meiosis-specific nuclear passenger protein is required for proper assembly of forespore membrane in fission yeast.

PubMed

Takaine, Masak; Imada, Kazuki; Numata, Osamu; Nakamura, Taro; Nakano, Kentaro

2014-10-15

Sporulation, gametogenesis in yeast, consists of meiotic nuclear division and spore morphogenesis. In the fission yeast Schizosaccharomyces pombe, the four haploid nuclei produced after meiosis II are encapsulated by the forespore membrane (FSM), which is newly synthesized from spindle pole bodies (SPBs) in the cytoplasm of the mother cell as spore precursors. Although the coordination between meiosis and FSM assembly is vital for proper sporulation, the underlying mechanism remains unclear. In the present study, we identified a new meiosis-specific protein Npg1, and found that it was involved in the efficient formation of spores and spore viability. The accumulation and organization of the FSM was compromised in npg1-null cells, leading to the error-prone envelopment of nuclei. Npg1 was first seen as internuclear dots and translocated to the SPBs before the FSM assembled. Genetic analysis revealed that Npg1 worked in conjunction with the FSM proteins Spo3 and Meu14. These results suggest a possible signaling link from the nucleus to the meiotic SPBs in order to associate the onset of FSM assembly with meiosis II, which ensures the successful partitioning of gametic nuclei. © 2014. Published by The Company of Biologists Ltd.

Abnormal Glucose Metabolism in Alzheimer’s Disease: Relation to Autophagy/Mitophagy and Therapeutic Approaches

PubMed Central

Banerjee, Kalpita; Munshi, Soumyabrata; Frank, David E.; Gibson, Gary E.

2015-01-01

Diminished glucose metabolism accompanies many neurodegenerative diseases including Alzheimer’s disease. An understanding of the relation of these metabolic changes to the disease will enable development of novel therapeutic strategies. Following a metabolic challenge, cells generally conserve energy to preserve viability. This requires activation of many cellular repair/regenerative processes such as mitophagy/autophagy and fusion/fission. These responses may diminish cell function in the long term. Prolonged fission induces mitophagy/autophagy which promotes repair but if prolonged progresses to mitochondrial degradation. Abnormal glucose metabolism alters protein signaling including the release of proteins from the mitochondria or migration of proteins from the cytosol to the mitochondria or nucleus. This overview provides an insight into the different mechanisms of autophagy/mitophagy and mitochondrial dynamics in response to the diminished metabolism that occurs with diseases, especially neurodegenerative diseases such as Alzheimer's disease. The review discusses multiple aspects of mitochondrial responses including different signaling proteins and pathways of mitophagy and mitochondrial biogenesis. Improving cellular bioenergetics and mitochondrial dynamics will alter protein signaling and improve cellular/mitochondrial repair and regeneration. An understanding of these changes will suggest new therapeutic strategies. PMID:26077923

Cobalt spin states and hyperfine interactions in LaCoO3 investigated by LDA+U calculations

NASA Astrophysics Data System (ADS)

Leighton, C.; Hsu, H.; Blaha, P.; Wentzcovitch, R. M.

2010-12-01

The spin states of cobalt ions in the bulk and epitaxial-thin-film lanthanum cobaltite (LaCoO3) have been controversial for years. The controversial point is mainly the presence of intermediate-spin (IS) Co in the temperature range of 0-85 K. In this region, bulk LaCoO3 experiences a crossover from a diamagnetic to a paramagnetic phase, and the thin-film LaCoO3 is ferromagnetic and insulator. An approach to probe the Co spin state is thus of interest. With a series of LDA+U calculations, we have demonstrated that the electric field gradient (EFG) at the Co nucleus can be used as a fingerprint to identify the spin state of the Co ion in each case. Therefore, in principle, the spin state of the Co ion can be unambiguously determined from nuclear magnetic resonance (NMR) spectra. Our calculations also suggest that the presence of IS Co in this temperature range is unlikely, based not only on its relatively higher energy, but also on its associated conducting band structure incompatible with the measured insulating conductivity. This work was primarily supported by the MRSEC Program of NSF under Awards Number DMR-0212302 and DMR-0819885, and partially supported by NSF under ATM-0428774 (V-Lab), EAR-1019853, and EAR-0810272. The computations were performed mainly at the Minnesota Supercomputing Institute (MSI).

Backbending in the {}_{90}^{223}{Th} nucleus: presentation of the consistency of two different experiments

NASA Astrophysics Data System (ADS)

Maquart, G.; Astier, A.; Ducoin, C.; Guinet, D.; Stézowski, O.; Augey, L.; Chaix, L.; Companis, I.; Dudouet, J.; Lehaut, G.; Mancuso, C.; Redon, N.; Vancraeyenest, A.

2017-06-01

The detailed level structure of {}223{Th} has been investigated in measurements of γ radiations following the fusion-evaporation channel of the {}208{Pb}{(}18{{O}},3n{)}223{Th} reaction at 85 MeV beam energy. The present data are extracted from two different experiments performed with the EUROBALL IV and JUROGAM II γ-ray detector array, respectively. The level structure has been extended up to spin 49/2 and 33 new γ-rays have been added using triple-γ coincidence data. The spins and parities of the newly observed states have been confirmed by angular distribution ratios. In addition to the two known yrast bands based on a K=5/2 configuration, a non-yrast band has been established up to spin 35/2. This observation has brought to light a sharp backbending occuring at the highest spins promoting the {}223{Th} as the heavier thorium isotope having an accident observed in its moment of inertia at high spin. We interpret this new structure as based on the same configuration as the yrast band in {}221{Th} having dominant K=1/2 contribution. At the highest spin a backbending occurs around a rotational frequency of {\\hslash }ω =0.23 {MeV}, very close to the one predicted in the {}222{Th} where a sharp transition to a reflection-symmetric shape is expected.

Elucidation of the mechanism of N-demethylation catalyzed by cytochrome P450 monooxygenase is facilitated by exploiting nitrogen-15 heavy isotope effects.

PubMed

Kwiecień, Renata A; Molinié, Roland; Paneth, Piotr; Silvestre, Virginie; Lebreton, Jacques; Robins, Richard J

2011-06-01

(15)N heavy isotope effects are especially useful when detail is sought pertaining to the reaction mechanism for the cleavage of a C-N bond. Their potential in assisting to describe the mechanism of N-demethylation of tertiary amines by the action of cytochrome P450 monooxygenase has been investigated. As a working model for the first step, oxidation of the N-methyl group to N-methoxyl, tropine and a cytochrome P450 monooxygenase reaction centre composed of a truncated heme with sulfhydryl as the axial ligand were used. It is apparent that this first step of the reaction proceeds via a hydrogen atom transfer mechanism. Transition states for this step are described for both the high spin ((4)TS(H)) and low spin ((2)TS(H)) pathways in both gas and solvation states. Hence, overall normal secondary (15)N KIE could be calculated for the reaction path modeled in the low spin state, and inverse for the reaction modeled in the high spin state. This partial reaction has been identified as the probable rate limiting step. The model for the second step, fission of the C-N bond, consisted of N-methoxylnortropine and two molecules of water. A transition state described for this step, TS(CN), gives a strongly inverse overall theoretical (15)N KIE. Copyright © 2011 Elsevier Inc. All rights reserved.

Efficient calculation of nuclear spin-rotation constants from auxiliary density functional theory.

PubMed

Zuniga-Gutierrez, Bernardo; Camacho-Gonzalez, Monica; Bendana-Castillo, Alfonso; Simon-Bastida, Patricia; Calaminici, Patrizia; Köster, Andreas M

2015-09-14

The computation of the spin-rotation tensor within the framework of auxiliary density functional theory (ADFT) in combination with the gauge including atomic orbital (GIAO) scheme, to treat the gauge origin problem, is presented. For the spin-rotation tensor, the calculation of the magnetic shielding tensor represents the most demanding computational task. Employing the ADFT-GIAO methodology, the central processing unit time for the magnetic shielding tensor calculation can be dramatically reduced. In this work, the quality of spin-rotation constants obtained with the ADFT-GIAO methodology is compared with available experimental data as well as with other theoretical results at the Hartree-Fock and coupled-cluster level of theory. It is found that the agreement between the ADFT-GIAO results and the experiment is good and very similar to the ones obtained by the coupled-cluster single-doubles-perturbative triples-GIAO methodology. With the improved computational performance achieved, the computation of the spin-rotation tensors of large systems or along Born-Oppenheimer molecular dynamics trajectories becomes feasible in reasonable times. Three models of carbon fullerenes containing hundreds of atoms and thousands of basis functions are used for benchmarking the performance. Furthermore, a theoretical study of temperature effects on the structure and spin-rotation tensor of the H(12)C-(12)CH-DF complex is presented. Here, the temperature dependency of the spin-rotation tensor of the fluorine nucleus can be used to identify experimentally the so far unknown bent isomer of this complex. To the best of our knowledge this is the first time that temperature effects on the spin-rotation tensor are investigated.

Investigation on the quasifission process by theoretical analysis of experimental data of fissionlike reaction products

NASA Astrophysics Data System (ADS)

Giardina, G.; Nasirov, A. K.; Mandaglio, G.; Curciarello, F.; De Leo, V.; Fazio, G.; Manganaro, M.; Romaniuk, M.; Saccá, C.

2011-02-01

The hindrance to complete fusion is a phenomenon presenting in the most part of the capture events in reactions with massive nuclei. This phenomenon is due to the onset of the quasifission process which competes with complete fusion during the evolution of the composed system formed at capture stage. The branching ratio between quasifission and complete fusion strongly depends from different characteristics of reacting nuclei in the entrance channel. The experimental and theoretical investigations of reaction dynamics connected with the formation of composed system is nowadays the main subject of the nuclear reactions. There is ambiguity in establishment of the reaction mechanism leading to the observed binary fissionlike fragments. The correct estimation of the fusion probability is important in planning experiments for the synthesis of superheavy elements. The experimental determination of evaporation residues only is not enough to restore the true reaction dynamics. The experimental observation of fissionlike fragments only cannot assure the correct distinguishing of products of the quasifission, fast fission, and fusion-fission processes which have overlapping in the mass (angular, kinetic energy) distributions of fragments. In this paper we consider a wide set of reactions (with different mass asymmetry and mass symmetry parameters) with the aim to explain the role played by many quantities on the reaction mechanisms. We also present the results of study of the 48Ca+249Bk reaction used to synthesize superheavy nuclei with Z = 117 by the determination of the evaporation residue cross sections and the effective fission barriers < Bf > of excited nuclei formed along the de-excitation cascade of the compound nucleus.

SPY: a new scission-point model based on microscopic inputs to predict fission fragment properties

NASA Astrophysics Data System (ADS)

Panebianco, Stefano; Dubray, Nöel; Goriely, Stéphane; Hilaire, Stéphane; Lemaître, Jean-François; Sida, Jean-Luc

2014-04-01

Despite the difficulty in describing the whole fission dynamics, the main fragment characteristics can be determined in a static approach based on a so-called scission-point model. Within this framework, a new Scission-Point model for the calculations of fission fragment Yields (SPY) has been developed. This model, initially based on the approach developed by Wilkins in the late seventies, consists in performing a static energy balance at scission, where the two fragments are supposed to be completely separated so that their macroscopic properties (mass and charge) can be considered as fixed. Given the knowledge of the system state density, averaged quantities such as mass and charge yields, mean kinetic and excitation energy can then be extracted in the framework of a microcanonical statistical description. The main advantage of the SPY model is the introduction of one of the most up-to-date microscopic descriptions of the nucleus for the individual energy of each fragment and, in the future, for their state density. These quantities are obtained in the framework of HFB calculations using the Gogny nucleon-nucleon interaction, ensuring an overall coherence of the model. Starting from a description of the SPY model and its main features, a comparison between the SPY predictions and experimental data will be discussed for some specific cases, from light nuclei around mercury to major actinides. Moreover, extensive predictions over the whole chart of nuclides will be discussed, with particular attention to their implication in stellar nucleosynthesis. Finally, future developments, mainly concerning the introduction of microscopic state densities, will be briefly discussed.

The Typical Number of Antiprotons Necessary to Heat the Hot Spot in the D-T Fuel Doped with U

NASA Astrophysics Data System (ADS)

Shmatov, M. L.

Fast ignition scenario with heating the hot spot by products of annihilation of antiprotons in the D-T fuel doped with U238 is considered. It is shown that in this scenario the hot spot is being heated effectively only by the fission fragments arising due to annihilation of the antiprotons on the nuclei of uranium. The presented model predicts that fast ignition can be provided by injection of (1.3 to 4.4) x 1015 antiprotons into the D-T fuel compressed to the density of about 200 g/cm3 and containing one nucleus of U238 per about one thousand nuclei of hydrogen isotopes.

Production of medical isotopes from a thorium target irradiated by light charged particles up to 70 MeV

NASA Astrophysics Data System (ADS)

Duchemin, C.; Guertin, A.; Haddad, F.; Michel, N.; Métivier, V.

2015-02-01

The irradiation of a thorium target by light charged particles (protons and deuterons) leads to the production of several isotopes of medical interest. Direct nuclear reaction allows the production of Protactinium-230 which decays to Uranium-230 the mother nucleus of Thorium-226, a promising isotope for alpha radionuclide therapy. The fission of Thorium-232 produces fragments of interest like Molybdenum-99, Iodine-131 and Cadmium-115g. We focus our study on the production of these isotopes, performing new cross section measurements and calculating production yields. Our new sets of data are compared with the literature and the last version of the TALYS code.

Production of medical isotopes from a thorium target irradiated by light charged particles up to 70 MeV.

PubMed

Duchemin, C; Guertin, A; Haddad, F; Michel, N; Métivier, V

2015-02-07

The irradiation of a thorium target by light charged particles (protons and deuterons) leads to the production of several isotopes of medical interest. Direct nuclear reaction allows the production of Protactinium-230 which decays to Uranium-230 the mother nucleus of Thorium-226, a promising isotope for alpha radionuclide therapy. The fission of Thorium-232 produces fragments of interest like Molybdenum-99, Iodine-131 and Cadmium-115g. We focus our study on the production of these isotopes, performing new cross section measurements and calculating production yields. Our new sets of data are compared with the literature and the last version of the TALYS code.

Highlights of modern nuclear structure.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Daly, P. J.

1998-09-11

Excitations of nuclei close to magic {sup 132}Sn have been investigated by analysis of fission product {gamma}-ray data measured at Eurogam II using a {sup 248}Cm source. Results for the N=82 isotopes up to {sup 136}Xe, for the one proton-one neutron nucleus {sup 134}Sb, and for the N=84 isotones {sup 134}Sn. {sup 135}Sb, and {sup 136}Te are summarized. The interpretation of the observed level spectra is mainly based on shell model calculations using empirical proton-proton interactions from {sup 134}Te, neutron-neutron interactions from is {sup 134}Sn, and proton-neutron interactions estimated (with scaling as A{sup {minus}1/3}) from the well-known {sup 210}Bi spectrum.

Velocity modulation spectroscopy of molecular ions II: The millimeter/submillimeter-wave spectrum of TiF + ( X3Φr)

NASA Astrophysics Data System (ADS)

Halfen, D. T.; Ziurys, L. M.

2006-11-01

The pure rotational spectrum of the molecular ion TiF + in its 3Φr ground state has been measured in the range 327-542 GHz using millimeter-wave direct absorption techniques combined with velocity modulation spectroscopy. TiF + was made in an AC discharge from a mixture of TiCl 4, F 2 in He, and argon. Ten transitions of this ion were recorded. In every transition, fluorine hyperfine interactions, as well as the fine structure splittings, were resolved. The fine structure pattern was found to be regular with almost equal spacing in frequency between the three spin components, in contrast to TiCl +, which is perturbed in the ground state. The data were fit with a case ( a) Hamiltonian and rotational, fine structure, and hyperfine constants were determined. The bond length established for TiF +, r0 = 1.7775 Å, was found to be shorter than that of TiF, r0 = 1.8342 Å—also established from mm-wave data. The hyperfine parameters determined are consistent with a δ1π1 electron configuration with the electrons primarily located on the titanium nucleus. The nuclear spin-orbit constant a indicates that the unpaired electrons are closer to the fluorine nucleus in TiF + relative to TiF, as expected with the decrease in bond length for the ion. The shorter bond distance is thought to arise from increased charge on the titanium nucleus as a result of a Ti 2+F - configuration. A similar decrease in bond length was found for TiCl + relative to TiCl.

High-spin terminating states in the N = 88 Ho 155 and Er 156 isotones

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rees, J. M.; Paul, E. S.; Simpson, J.

2015-05-01

The Sn-124(Cl-37, 6n gamma) fusion-evaporation reaction at a bombarding energy of 180 MeV has been used to significantly extend the excitation level scheme of Ho-155(67)88. The collective rotational behavior of this nucleus breaks down above spin I similar to 30 and a fully aligned noncollective (band terminating) state has been identified at I-pi = 79/2(-). Comparison with cranked Nilsson-Strutinsky calculations also provides evidence for core-excited noncollective states at I-pi = 87/2(-) and (89/2(+)) involving particle-hole excitations across the Z = 64 shell gap. A similar core-excited state in Er-156(68)88 at I-pi = (46(+)) is also presented.

Need of a consistent and convenient nucleus identification in ENDF files for the automatic construction of the depletion chains

NASA Astrophysics Data System (ADS)

Mosca, Pietro; Mounier, Claude

2016-03-01

The automatic construction of evolution chains recently implemented in GALILEE system is based on the analysis of several ENDF files : the multigroup production cross sections present in the GENDF files processed by NJOY from the ENDF evaluation, the decay file and the fission product yields (FPY) file. In this context, this paper highlights the importance of the nucleus identification to properly interconnect the data mentioned above. The first part of the paper describes the present status of the nucleus identification among the several ENDF files focusing, in particular, on the use of the excited state number and of the isomeric state number. The second part reviews the problems encountered during the automatic construction of the depletion chains using recent ENDF data. The processing of the JEFF-3.1.1, ENDF/B-VII.0 (decay and FPY) and the JEFF-3.2 (production cross section) points out problems about the compliance or not of the nucleus identifiers with the ENDF-6 format and sometimes the inconsistencies among the various ENDF files. In addition, the analysis of EAF-2003 and EAF-2010 shows some incoherence between the ZA product identifier and the reaction identifier MT for the reactions (n, pα) and (n, 2np). As a main result of this work, our suggestion is to change the ENDF format using systematically the isomeric state number to identify the nuclei. This proposal is already compliant to a huge amount ENDF data that are not in agreement with the present ENDF format. This choice is the most convenient because, ultimately, it allows one to give human readable names to the nuclei of the depletion chains.

Nuclear-driven electron spin rotations in a coupled silicon quantum dot and single donor system

NASA Astrophysics Data System (ADS)

Harvey-Collard, Patrick; Jacobson, Noah Tobias; Rudolph, Martin; Ten Eyck, Gregory A.; Wendt, Joel R.; Pluym, Tammy; Lilly, Michael P.; Pioro-Ladrière, Michel; Carroll, Malcolm S.

Single donors in silicon are very good qubits. However, a central challenge is to couple them to one another. To achieve this, many proposals rely on using a nearby quantum dot (QD) to mediate an interaction. In this work, we demonstrate the coherent coupling of electron spins between a single 31P donor and an enriched 28Si metal-oxide-semiconductor few-electron QD. We show that the electron-nuclear spin interaction can drive coherent rotations between singlet and triplet electron spin states. Moreover, we are able to tune electrically the exchange interaction between the QD and donor electrons. The combination of single-nucleus-driven rotations and voltage-tunable exchange provides all elements for future all-electrical control of a spin qubit, and requires only a single dot and no additional magnetic field gradients. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's National Nuclear Security Administration under Contract DE-AC04-94AL85000.

Polarization-polarization correlation measurement --- Experimental test of the PPCO methods

NASA Astrophysics Data System (ADS)

Droste, Ch.; Starosta, K.; Wierzchucka, A.; Morek, T.; Rohoziński, S. G.; Srebrny, J.; Wesolowski, E.; Bergstrem, M.; Herskind, B.

1998-04-01

A significant fraction of modern multidetector arrays used for "in-beam" gamma-ray spectroscopy consist of a detectors which are sensitive to linear polarization of gamma quanta. This yields the opportunity to carry out correlation measurements between the gamma rays registered in polarimeters to get information concerning spins and parities of excited nuclear states. The aim of the present work was to study the ability of the polarization- polarization correlation method (the PPCO method). The correlation between the linear polarization of one gamma quantum and the polarization of the second quantum emitted in a cascade from an oriented nucleus (due to a heavy ion reaction) was studied in detail. The appropriate formulae and methods of analysis are presented. The experimental test of the method was performed using the EUROGAM II array. The CLOVER detectors are the parts of the array used as polarimeters. The ^164Yb nucleus was produced via the ^138Ba(^30Si, 4n) reaction. It was found that the PPCO method together with the standard DCO analysis and the polarization- direction correlation method (PDCO) can be helpful for spin, parity and multipolarity assignments. The results suggest that the PPCO method can be applied to modern spectrometers in which a large number of detectors (e.g. CLOVER) are sensitive to polarization of gamma rays.

Spin-orbit coupling calculations with the two-component normalized elimination of the small component method

NASA Astrophysics Data System (ADS)

Filatov, Michael; Zou, Wenli; Cremer, Dieter

2013-07-01

A new algorithm for the two-component Normalized Elimination of the Small Component (2cNESC) method is presented and tested in the calculation of spin-orbit (SO) splittings for a series of heavy atoms and their molecules. The 2cNESC is a Dirac-exact method that employs the exact two-component one-electron Hamiltonian and thus leads to exact Dirac SO splittings for one-electron atoms. For many-electron atoms and molecules, the effect of the two-electron SO interaction is modeled by a screened nucleus potential using effective nuclear charges as proposed by Boettger [Phys. Rev. B 62, 7809 (2000), 10.1103/PhysRevB.62.7809]. The use of the screened nucleus potential for the two-electron SO interaction leads to accurate spinor energy splittings, for which the deviations from the accurate Dirac Fock-Coulomb values are on the average far below the deviations observed for other effective one-electron SO operators. For hydrogen halides HX (X = F, Cl, Br, I, At, and Uus) and mercury dihalides HgX2 (X = F, Cl, Br, I) trends in spinor energies and SO splittings as obtained with the 2cNESC method are analyzed and discussed on the basis of coupling schemes and the electronegativity of X.

New excitations in Ba 142 and Ce 144 : Evolution of γ bands in the N = 86 isotones

DOE PAGES

Naidja, H.; Nowacki, F.; Bounthong, B.; ...

2017-06-02

New excited states in 142Ba and 144Ce are investigated by means of prompt γ-ray spectroscopy of the radiation following spontaneous fission of 252Cf. Measurements of angular correlations and the observed branchings allowed the assignment of spins and parities with confidence. The new measurements are reinforced by shell-model calculations where energy levels, electric transitions, and magnetic moments are consistent with experimental data. Lastly, the presence of collectivity in the N = 86 isotones is confirmed by clear signatures of soft triaxial γ bands in both nuclei.

Scissors Mode of 162 Dy Studied from Resonance Neutron Capture

DOE PAGES

Baramsai, B.; Bečvář, F.; Bredeweg, T. A.; ...

2015-05-28

Multi-step cascade γ-ray spectra from the neutron capture at isolated resonances of 161Dy nucleus were measured at the LANSCE/DANCE time-of-flight facility in Los Alamos National Laboratory. The objectives of this experiment were to confirm and possibly extend the spin assignment of s-wave neutron resonances and get new information on photon strength functions with emphasis on the role of the M1 scissors mode vibration. The preliminary results show that the scissors mode plays a significant role in all transitions between accessible states of the studied nucleus. The photon strength functions describing well our data are compared to results from 3He-induced reactions,more » (n,γ) experiments on Gd isotopes, and (γ,γ’) reactions.« less

YORP and collisional shaping of the sub-populations, rotation rate and size-frequency distributions in the main-belt

NASA Astrophysics Data System (ADS)

Rossi, A.; Marzari, F.; Scheeres, D.; Jacobson, S.; Davis, D.

In the last several years a comprehensive asteroid-population-evolution model was developed incorporating both the YORP effect and collisional evolution \\citep{rossi_2009}, \\citep{marz_2011}, \\citep{jac_mnras}. From the results of this model we were able to match the observed main belt rotation rate distribution and to give a first plausible explanation of the observed excess of slow rotators, through a random walk-like evolution of the spin, induced by repeated collisions with small projectiles. Moreover, adding to the model the rotational fission hypothesis (i.e. when the rotation rate exceeds a critical value, erosion and binary formation occur; \\citealt{sch_2007}) and binary-asteroid evolution \\citep{jac_sch}, we first showed that the YORP-induced rotational-fission hypothesis has strong repercussions for the small size end of the main-belt asteroid size-frequency distribution. We also concluded that this hypothesis is consistent with observed asteroid-population statistics and with the observed sub-populations of binary asteroids, asteroid pairs and contact binaries. An overview of the results obtained, the modelling uncertainties and the ongoing work will be given.

Hyperfine interaction mechanism of magnetic field effects in sequential fluorophore and exciplex fluorescence.

PubMed

Dodin, Dmitry V; Ivanov, Anatoly I; Burshtein, Anatoly I

2013-03-28

The magnetic field effect on the fluorescence of the photoexcited electron acceptor, (1)A∗, and the exciplex, (1)[D(+δ)A(-δ)] formed at contact of (1)A∗ with an electron donor (1)D, is theoretically explored in the framework of Integral Encounter Theory. It is assumed that the excited fluorophore is equilibrated with the exciplex that reversibly dissociates into the radical-ion pair. The magnetic field sensitive stage is the spin conversion in the resulting geminate radical-ion pair, (1, 3)[D(+)...A(-)] that proceeds due to hyperfine interaction. We confirm our earlier conclusion (obtained with a rate description of spin conversion) that in the model with a single nucleus spin 1/2 the magnitude of the Magnetic Field Effect (MFE) also vanishes in the opposite limits of low and high dielectric permittivity of the solvent. Moreover, it is shown that MFE being positive at small hyperfine interaction A, first increases with A but approaching the maximum starts to decrease and even changes the sign.

First observation of rotational structures in Re 168

DOE PAGES

Hartley, D. J.; Janssens, R. V. F.; Riedinger, L. L.; ...

2016-11-30

We assigned first rotational sequences to the odd-odd nucleus 168Re. Coincidence relationships of these structures with rhenium x rays confirm the isotopic assignment, while arguments based on the γ-ray multiplicity (K-fold) distributions observed with the new bands lead to the mass assignment. Configurations for the two bands were determined through analysis of the rotational alignments of the structures and a comparison of the experimental B(M1)/B(E2) ratios with theory. Tentative spin assignments are proposed for the πh 11/2νi 13/2 band, based on energy level systematics for other known sequences in neighboring odd-odd rhenium nuclei, as well as on systematics seen formore » the signature inversion feature that is well known in this region. Furthermore, the spin assignment for the πh 11/2ν(h 9/2/f 7/2) structure provides additional validation of the proposed spins and configurations for isomers in the 176Au → 172Ir → 168Re α-decay chain.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hartley, D. J.; Janssens, R. V. F.; Riedinger, L. L.

We assigned first rotational sequences to the odd-odd nucleus 168Re. Coincidence relationships of these structures with rhenium x rays confirm the isotopic assignment, while arguments based on the γ-ray multiplicity (K-fold) distributions observed with the new bands lead to the mass assignment. Configurations for the two bands were determined through analysis of the rotational alignments of the structures and a comparison of the experimental B(M1)/B(E2) ratios with theory. Tentative spin assignments are proposed for the πh 11/2νi 13/2 band, based on energy level systematics for other known sequences in neighboring odd-odd rhenium nuclei, as well as on systematics seen formore » the signature inversion feature that is well known in this region. Furthermore, the spin assignment for the πh 11/2ν(h 9/2/f 7/2) structure provides additional validation of the proposed spins and configurations for isomers in the 176Au → 172Ir → 168Re α-decay chain.« less

High spin states in 164Lu

NASA Astrophysics Data System (ADS)

Juneja, P.; Gupta, S. L.; Pancholi, S. C.; Kumar, Ashok; Mehta, D.; Chaturvedi, L.; Katoch, S. K.; Malik, S.; Shanker, G.; Bhowmik, R. K.; Muralithar, S.; Rodrigues, G.; Singh, R. P.

1996-03-01

High spin states in the odd-odd 164Lu nucleus have been investigated for the first time, through in-beam gamma-ray spectroscopy, following the 150Sm(19F,5n) reaction at beam energy Elab=105 MeV. Four bands, including two signature split bands are identified. The interpretation of the experimental results is discussed in comparison with the existing data in the neighboring nuclei and in the framework of the cranked shell model. The πh11/2⊗νi13/2 yrast band exhibits anomalous signature splitting and signature inversion is observed at a spin of 18ħ. This provides the missing datum for the systematics of staggering and signature inversion for the neighboring odd-odd N=93 isotones and supports the predictions of angular-momentum projection calculations by Hara and Sun. In the second signature split πh 11/2h9/2 band, the AB neutron crossing occurs at a rotational frequency of ~0.29 MeV. This is indicative of the disappearance of the blocking effect of the odd neutron.

Magnetic resonance imaging of (1)H long lived states derived from parahydrogen induced polarization in a clinical system.

PubMed

Graafen, Dirk; Franzoni, María Belén; Schreiber, Laura M; Spiess, Hans W; Münnemann, Kerstin

2016-01-01

Hyperpolarization is a powerful tool to overcome the low sensitivity of nuclear magnetic resonance (NMR). However, applications are limited due to the short lifetime of this non equilibrium spin state caused by relaxation processes. This issue can be addressed by storing hyperpolarization in slowly decaying singlet spin states which was so far mostly demonstrated for non-proton spin pairs, e.g. (13)C-(13)C. Protons hyperpolarized by parahydrogen induced polarization (PHIP) in symmetrical molecules, are very well suited for this strategy because they naturally exhibit a long-lived singlet state. The conversion of the NMR silent singlet spin state to observable magnetization can be achieved by making use of singlet-triplet level anticrossings. In this study, a low-power radiofrequency pulse sequence is used for this purpose, which allows multiple successive singlet-triplet conversions. The generated magnetization is used to record proton images in a clinical magnetic resonance imaging (MRI) system, after 3min waiting time. Our results may open unprecedented opportunities to use the standard MRI nucleus (1)H for e.g. metabolic imaging in the future. Copyright © 2016. Published by Elsevier Inc.

Final state interactions and the extraction of neutron single spin asymmetries from semi-inclusive deep-inelastic scattering by a transversely polarized 3He target

NASA Astrophysics Data System (ADS)

Del Dotto, A.; Kaptari, L. P.; Pace, E.; Salmè, G.; Scopetta, S.

2017-12-01

The semi-inclusive deep-inelastic electron scattering off transversely polarized 3He, i.e., the process e +3He ⃗→e'+h +X , with h being a detected fast hadron, is studied beyond the plane-wave impulse approximation. To this end, a distorted spin-dependent spectral function of a nucleon inside an A =3 nucleus is actually evaluated through a generalized eikonal approximation, in order to take into account the final state interactions between the hadronizing system and the (A -1 ) nucleon spectator one. Our realistic description of both nuclear target and final state is a substantial step forward for achieving a reliable extraction of the Sivers and Collins single spin asymmetries of the free neutron. To illustrate how and to what extent the model dependence due to the treatment of the nuclear effects is under control, we apply our approach to the extraction procedure of the neutron single spin asymmetries from those measured for 3He for values of the kinematical variables relevant both for forthcoming experiments at Jefferson Laboratory and, with an exploratory purpose, for the future Electron Ion Collider.

Nanosecond lifetime measurements of Iπ=9/2- intrinsic excited states and low-lying B(E1) strengths in 183Re using combined HPGe-LaBr3 coincidence spectroscopy

NASA Astrophysics Data System (ADS)

Gurgi, L. A.; Regan, P. H.; Daniel, T.; Podolyák, Zs.; Bruce, A. M.; Mason, P. J. R.; Mǎrginean, N.; Mǎrginean, R.; Werner, V.; Alharbi, T.; Alkhomashi, N.; Bajoga, A. D.; Britton, R.; Cǎta-Danil, I.; Carroll, R. J.; Deleanu, D.; Bucurescu, D.; Florea, N.; Gheorghe, I.; Ghita, D. G.; Glodariu, T.; Lice, R.; Mihai, C.; Mulholland, K. F.; Negret, A.; Olacel, A.; Roberts, O. J.; Sava, T.; Söderström, P.-A.; Stroe, L.; Suvaila, R.; Toma, S.; Wilson, E.; Wood, R. T.

2017-08-01

This paper presents precision measurements of electromagnetic decay probabilities associated with electric dipole transitions in the prolate-deformed nucleus 183Re. The nucleus of interest was formed using the fusion evaporation reaction 180Hf(7Li,4n)183Re at a beam energy of 30 MeV at the tandem accelerator at the HH-IFIN Institute, Bucharest Romania. Coincident decay gamma rays from near-yrast cascades were detected using the combined HPGe-LaBr3 detector array ROSPHERE. The time differences between cascade gamma rays were measured using the LaBr3 detectors to determine the half-lives of the two lowest lying spin-parity 9/2- states at excitation energies of 496 and 617 keV to be 5.65(5) and 2.08(3) ns respectively. The deduced E1 transition rates from these two states are discussed in terms of the K-hindrance between the low-lying structures in this prolate-deformed nucleus.

Global optical model potential for A=3 projectiles

NASA Astrophysics Data System (ADS)

Pang, D. Y.; Roussel-Chomaz, P.; Savajols, H.; Varner, R. L.; Wolski, R.

2009-02-01

A global optical model potential (GDP08) for He3 projectiles has been obtained by simultaneously fitting the elastic scattering data of He3 from targets of 40⩽AT⩽209 at incident energies of 30⩽Einc⩽217 MeV. Uncertainties and correlation coefficients between the global potential parameters were obtained by using the bootstrap statistical method. GDP08 was found to satisfactorily account for the elastic scattering of H3 as well, which makes it a global optical potential for the A=3 nuclei. Optical model calculations using the GDP08 global potential are compared with the experimental angular distributions of differential cross sections for He3-nucleus and H3-nucleus scattering from different targets of 6⩽AT⩽232 at incident energies of 4⩽Einc⩽450 MeV. The optical potential for the doubly-magic nucleus Ca40, the low-energy correction to the real potential for nuclei with 58≲AT≲120 at Einc<30 MeV, the comparison with double-folding model calculations and the CH89 potential, and the spin-orbit potential parameters are discussed.

Disaggregation of small, cohesive rubble pile asteroids due to YORP

NASA Astrophysics Data System (ADS)

Scheeres, D. J.

2018-04-01

The implication of small amounts of cohesion within relatively small rubble pile asteroids is investigated with regard to their evolution under the persistent presence of the YORP effect. We find that below a characteristic size, which is a function of cohesive strength, density and other properties, rubble pile asteroids can enter a "disaggregation phase" in which they are subject to repeated fissions after which the formation of a stabilizing binary system is not possible. Once this threshold is passed rubble pile asteroids may be disaggregated into their constituent components within a finite time span. These constituent components will have their own spin limits - albeit potentially at a much higher spin rate due to the greater strength of a monolithic body. The implications of this prediction are discussed and include modification of size distributions, prevalence of monolithic bodies among meteoroids and the lifetime of small rubble pile bodies in the solar system. The theory is then used to place constraints on the strength of binary asteroids characterized as a function of their type.

New isomer and decay half-life of {sup 115}Ru

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kurpeta, J.; Plochocki, A.; Rissanen, J.

2010-12-15

Exotic, neutron-rich nuclei of mass A=115 produced in proton-induced fission of {sup 238}U were extracted using the IGISOL mass separator. The beam of isobars was transferred to the JYFLTRAP Penning trap system for further separation to the isotopic level. Monoisotopic samples of {sup 115}Ru nuclei were used for {gamma}and {beta} coincidence spectroscopy. In {sup 115}Ru we have observed excited levels, including an isomer with a half-life of 76(6) ms and (7/2{sup -}) spin and parity. The first excited 61.7-keV level in {sup 115}Ru with spins and parity (3/2{sup +}) may correspond to an oblate 3/2{sup +}[431] Nilsson orbital. A half-lifemore » of 318(19) ms for the {beta}{sup -} decay of the (1/2{sup +}) ground state in {sup 115}Ru has been firmly established in two independent measurements, a value which is significantly shorter than that previously reported.« less

EXCITATION OF LEVELS IN Li$sup 7$ BY INELASTIC ELECTRON SCATTERING

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bernheim, M; Bishop, G R

1963-07-15

Cross sections for the excitation of some levels in Li/sup 7/ up to 8- Mev excitation energy were measured by the iiielastic scattering of electrons for a variety of incident electron energies and scatiering angles. The cross section calculated in first Dorn approximation is expected to be valid for this nucleus. The calculated angular distribution is given for different spin and parity and for different levels of excitation. (R.E.U.)

Frequency Conversion of Single Photons: Physics, Devices, and Applications

DTIC Science & Technology

2012-07-01

Ginzton lab who have also been instrumental have been Steve Sensarn, Il-Woong Jung , Kelley Rivoire, Gary Shambat, Sonia Buckley, Kiarash Aghaie, Na...My initial projects in the Fejer group were focused on modeling a synchronously pumped OPO for terahertz generation. A ps-pulsed 1064-nm laser...detection of the spin state of a single nucleus in silicon. Physical Review B, 69(12):125306, March 2004. BIBLIOGRAPHY 151 [116] Carl A. Kocher and

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zuniga-Gutierrez, Bernardo, E-mail: bzuniga.51@gmail.com; Camacho-Gonzalez, Monica; Bendana-Castillo, Alfonso

The computation of the spin-rotation tensor within the framework of auxiliary density functional theory (ADFT) in combination with the gauge including atomic orbital (GIAO) scheme, to treat the gauge origin problem, is presented. For the spin-rotation tensor, the calculation of the magnetic shielding tensor represents the most demanding computational task. Employing the ADFT-GIAO methodology, the central processing unit time for the magnetic shielding tensor calculation can be dramatically reduced. In this work, the quality of spin-rotation constants obtained with the ADFT-GIAO methodology is compared with available experimental data as well as with other theoretical results at the Hartree-Fock and coupled-clustermore » level of theory. It is found that the agreement between the ADFT-GIAO results and the experiment is good and very similar to the ones obtained by the coupled-cluster single-doubles-perturbative triples-GIAO methodology. With the improved computational performance achieved, the computation of the spin-rotation tensors of large systems or along Born-Oppenheimer molecular dynamics trajectories becomes feasible in reasonable times. Three models of carbon fullerenes containing hundreds of atoms and thousands of basis functions are used for benchmarking the performance. Furthermore, a theoretical study of temperature effects on the structure and spin-rotation tensor of the H{sup 12}C–{sup 12}CH–DF complex is presented. Here, the temperature dependency of the spin-rotation tensor of the fluorine nucleus can be used to identify experimentally the so far unknown bent isomer of this complex. To the best of our knowledge this is the first time that temperature effects on the spin-rotation tensor are investigated.« less

Measurement of the magnetic interaction between two bound electrons of two separate ions.

PubMed

Kotler, Shlomi; Akerman, Nitzan; Navon, Nir; Glickman, Yinnon; Ozeri, Roee

2014-06-19

Electrons have an intrinsic, indivisible, magnetic dipole aligned with their internal angular momentum (spin). The magnetic interaction between two electronic spins can therefore impose a change in their orientation. Similar dipolar magnetic interactions exist between other spin systems and have been studied experimentally. Examples include the interaction between an electron and its nucleus and the interaction between several multi-electron spin complexes. The challenge in observing such interactions for two electrons is twofold. First, at the atomic scale, where the coupling is relatively large, it is often dominated by the much larger Coulomb exchange counterpart. Second, on scales that are substantially larger than the atomic, the magnetic coupling is very weak and can be well below the ambient magnetic noise. Here we report the measurement of the magnetic interaction between the two ground-state spin-1/2 valence electrons of two (88)Sr(+) ions, co-trapped in an electric Paul trap. We varied the ion separation, d, between 2.18 and 2.76 micrometres and measured the electrons' weak, millihertz-scale, magnetic interaction as a function of distance, in the presence of magnetic noise that was six orders of magnitude larger than the magnetic fields the electrons apply on each other. The cooperative spin dynamics was kept coherent for 15 seconds, during which spin entanglement was generated, as verified by a negative measured value of -0.16 for the swap entanglement witness. The sensitivity necessary for this measurement was provided by restricting the spin evolution to a decoherence-free subspace that is immune to collective magnetic field noise. Our measurements show a d(-3.0(4)) distance dependence for the coupling, consistent with the inverse-cube law.

Site-resolved multiple-quantum filtered correlations and distance measurements by magic-angle spinning NMR: Theory and applications to spins with weak to vanishing quadrupolar couplings

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eliav, U., E-mail: amirgo@tau.ac.il, E-mail: eliav@tau.ac.il; Haimovich, A.; Goldbourt, A., E-mail: amirgo@tau.ac.il, E-mail: eliav@tau.ac.il

2016-01-14

We discuss and analyze four magic-angle spinning solid-state NMR methods that can be used to measure internuclear distances and to obtain correlation spectra between a spin I = 1/2 and a half-integer spin S > 1/2 having a small quadrupolar coupling constant. Three of the methods are based on the heteronuclear multiple-quantum and single-quantum correlation experiments, that is, high rank tensors that involve the half spin and the quadrupolar spin are generated. Here, both zero and single-quantum coherence of the half spins are allowed and various coherence orders of the quadrupolar spin are generated, and filtered, via active recoupling ofmore » the dipolar interaction. As a result of generating coherence orders larger than one, the spectral resolution for the quadrupolar nucleus increases linearly with the coherence order. Since the formation of high rank tensors is independent of the existence of a finite quadrupolar interaction, these experiments are also suitable to materials in which there is high symmetry around the quadrupolar spin. A fourth experiment is based on the initial quadrupolar-driven excitation of symmetric high order coherences (up to p = 2S, where S is the spin number) and subsequently generating by the heteronuclear dipolar interaction higher rank (l + 1 or higher) tensors that involve also the half spins. Due to the nature of this technique, it also provides information on the relative orientations of the quadrupolar and dipolar interaction tensors. For the ideal case in which the pulses are sufficiently strong with respect to other interactions, we derive analytical expressions for all experiments as well as for the transferred echo double resonance experiment involving a quadrupolar spin. We show by comparison of the fitting of simulations and the analytical expressions to experimental data that the analytical expressions are sufficiently accurate to provide experimental {sup 7}Li–{sup 13}C distances in a complex of lithium, glycine, and water. Discussion of the regime for which such an approach is valid is given.« less

MadDM: Computation of dark matter relic abundance

NASA Astrophysics Data System (ADS)

Backović, Mihailo; Kong, Kyoungchul; McCaskey, Mathew

2017-12-01

MadDM computes dark matter relic abundance and dark matter nucleus scattering rates in a generic model. The code is based on the existing MadGraph 5 architecture and as such is easily integrable into any MadGraph collider study. A simple Python interface offers a level of user-friendliness characteristic of MadGraph 5 without sacrificing functionality. MadDM is able to calculate the dark matter relic abundance in models which include a multi-component dark sector, resonance annihilation channels and co-annihilations. The direct detection module of MadDM calculates spin independent / spin dependent dark matter-nucleon cross sections and differential recoil rates as a function of recoil energy, angle and time. The code provides a simplified simulation of detector effects for a wide range of target materials and volumes.

Elastic scattering of spin-polarized electrons and positrons from 23Na nuclei

NASA Astrophysics Data System (ADS)

Jakubassa-Amundsen, D. H.

2018-07-01

Differential cross sections and polarization correlations for the scattering of relativistic spin-polarized leptons from unpolarized ground-state sodium nuclei are calculated within the distorted-wave Born approximation (DWBA). Various nuclear ground-state charge distributions are probed. Besides potential scattering, also electric C2 and magnetic M1 and M3 transitions are taken into account. It is shown that even for a light nucleus such as 23Na there are considerable electron-positron differences at high collision energies and large scattering angles. In particular, the symmetry of the Sherman function with respect to a global sign change, as predicted by the second-order Born approximation when replacing electrons by positrons, is broken whenever the diffraction structures come into play beyond 100 MeV.

Spin-flip isovector giant resonances from the 90Zr(n,p)90Y reaction at 198 MeV

NASA Astrophysics Data System (ADS)

Raywood, K. J.; Spicer, B. M.; Yen, S.; Long, S. A.; Moinester, M. A.; Abegg, R.; Alford, W. P.; Celler, A.; Drake, T. E.; Frekers, D.; Green, P. E.; Häusser, O.; Helmer, R. L.; Henderson, R. S.; Hicks, K. H.; Jackson, K. P.; Jeppesen, R. G.; King, J. D.; King, N. S.; Miller, C. A.; Officer, V. C.; Schubank, R.; Shute, G. G.; Vetterli, M.; Watson, J.; Yavin, A. I.

1990-06-01

Doubly differential cross sections of the reaction 90Zr(n,p)90Y have been measured at 198 MeV for excitations up to 38 MeV in the residual nucleus. An overall resolution of 1.3 MeV was achieved. The spectra show qualitative agreement in shape and magnitude with recent random phase approximation calculations; however, all of the calculations underestimate the high excitation region of the spectra. A multipole decomposition of the data has been performed using differential cross sections calculated in the distorted-wave impulse approximation. An estimate of the Gamow-Teller strength in the reaction is given. The isovector spin-flip dipole giant resonance has been identified and there is also an indication of isovector monopole strength.

Evolution of single-particle structure and beta-decay near 78Ni

NASA Astrophysics Data System (ADS)

Borzov, I. N.

2012-12-01

The extended self-consistent beta-decay model has been applied for bet-decay rates and delayed neutron emission probabilities of spherical neutron-rich isotopes near the r-process paths. Unlike a popular global FRDM+RPA model, in our fully microscopic approach, the Gamow-Teller and first-forbidden decays are treated on the same footing. The model has been augmented by blocking of the odd particle in order to account for important ground-state spin-parity inversion effect which has been shown to exist in the region of the most neutron-rich doubly-magic nucleus 78Ni. Finally, a newly developed form of density functional DF3a has been employed which gives a better spin-orbit splitting due to the modified tensor components of the density functional.

Unambiguously identifying spin states of transition-metal ions in the Earth (Invited)

NASA Astrophysics Data System (ADS)

Hsu, H.

2010-12-01

The spin state of a transition-metal ion in crystalline solids, defined by the number of unpaired electrons in the ion’s incomplete 3d shell, may vary with many factors, such as temperature, pressure, strain, and the local atomic configuration, to name a few. Such a phenomenon, known as spin-state crossover, plays a crucial role in spintronic materials. Recently, the pressure-induced spin-state crossover in iron-bearing minerals has been recognized to affect the minerals’ structural and elastic properties. However, the detailed mechanism of such crossover in iron-bearing magnesium silicate perovskite, the most abundant mineral in the Earth, remains unclear. A significant part of this confusion arises from the difficulty in reliably extracting the spin state from experiments. For the same reason, the thermally-induced spin-state crossover in lanthanum cobaltite (LaCoO3) has been controversial for more than four decades. In this talk, I will discuss how first-principle calculations can help clarifying these long-standing controversies. In addition to the total energy, equation of state, and elastic properties of each spin state, first-principle calculations also predict the electric field gradient (EFG) at the nucleus of each transition-metal ion. Our calculations showed that the nuclear EFG, a quantity that can be measured via Mössbauer or nuclear magnetic resonance (NMR) spectroscopy, depends primarily on the spin state, irrespective of the concentration or configuration of transition-metal ions. Such robustness makes EFG a unique fingerprint to identify the spin state. The combination of first-principle calculations and Mössbauer/NMR spectroscopy can therefore be a reliable and efficient approach in tackling spin-state crossover problems in the Earth. This work was primarily supported by the MRSEC Program of NSF under Awards Number DMR-0212302 and DMR-0819885, and partially supported by NSF under ATM-0428774 (V-Lab), EAR-1019853, and EAR-0810272. The computations were performed mainly at the Minnesota Supercomputing Institute (MSI).

Nuclear relaxation in an electric field enables the determination of isotropic magnetic shielding

DOE Office of Scientific and Technical Information (OSTI.GOV)

Garbacz, Piotr, E-mail: pgarbacz@chem.uw.edu.pl

2016-08-14

It is shown that in contrast to the case of nuclear relaxation in a magnetic field B, simultaneous application of the magnetic field B and an additional electric field E causes transverse relaxation of a spin-1/2 nucleus with the rate proportional to the square of the isotropic part of the magnetic shielding tensor. This effect can contribute noticeably to the transverse relaxation rate of heavy nuclei in molecules that possess permanent electric dipole moments. Relativistic quantum mechanical computations indicate that for {sup 205}Tl nucleus in a Pt-Tl bonded complex, Pt(CN){sub 5}Tl, the transverse relaxation rate induced by the electric fieldmore » is of the order of 1 s{sup −1} at E = 5 kV/mm and B = 10 T.« less

What perspectives for the synthesis of heavier superheavy nuclei? Results and comparison with models

NASA Astrophysics Data System (ADS)

Mandaglio, G.; Nasirov, A. K.; Curciarello, F.; De Leo, V.; Romaniuk, M.; Fazio, G.; Giardina, G.

2013-03-01

The possibility to synthesize heavier superheavy elements in massive nuclei reactions is strongly limited by the hindrance to complete fusion of reacting nuclei: due to the onset of the quasifission process in the entrance channel, which competes with complete fusion, and by strong increase of the fission yield along the de-excitation cascade of the compound nucleus in comparison to the evaporation residue formation. We present a wide and detailed procedure allowing us to describe the experimental results (evaporation residue nuclei and fissionlike products) in the mass asymmetric and symmetric reactions. Very reliable estimations and perspectives for the synthesis of superheavy elements in many massive nuclei reactions up to Z = 120 and eventually also for Z > 120 have been obtained.

Nucleus Z=126 with magic neutron number N=184 may be related to the measured Maruhn-Greiner maximum at A/2=155 from compound nuclei at low energy nuclear reactions

NASA Astrophysics Data System (ADS)

Prelas, M. A.; Hora, H.; Miley, G. H.

2014-07-01

Evaluation of nuclear binding energies from theory close to available measurements of a very high number of superheavy elements (SHE) based on α-decay energies Qα, arrived at a closing shell with a significant neutron number 184. Within the option of several discussed magic numbers for protons of around 120, Bagge's numbers 126 and 184 fit well and are supported by the element generation measurements by low energy nuclear reactions (LENR) discovered in deuterium loaded host metals. These measurements were showing a Maruhn-Greiner maximum from fission of compound nuclei in an excited state with double magic numbers for mutual confirmation.

Stochastic YORP On Real Asteroid Shapes

NASA Astrophysics Data System (ADS)

McMahon, Jay W.

2015-05-01

Since its theoretical foundation and subsequent observational verification, the YORP effect has been understood to be a fundamental process that controls the evolution of small asteroids in the inner solar system. In particular, the coupling of the YORP and Yarkovsky effects are hypothesized to be largely responsible for the transport of asteroids from the main belt to the inner solar system populations. Furthermore, the YORP effect is thought to lead to rotational fission of small asteroids, which leads to the creation of multiple asteroid systems, contact binary asteroids, and asteroid pairs. However recent studies have called into question the ability of YORP to produce these results. In particular, the high sensitivity of the YORP coefficients to variations in the shape of an asteroid, combined with the possibility of a changing shape due to YORP accelerated spin rates can combine to create a stochastic YORP coefficient which can arrest or change the evolution of a small asteroid's spin state. In this talk, initial results are presented from new simulations which comprehensively model the stochastic YORP process. Shape change is governed by the surface slopes on radar based asteroid shape models, where the highest slope regions change first. The investigation of the modification of YORP coefficients and subsequent spin state evolution as a result of this dynamically influenced shape change is presented and discussed.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Matsuta, K.; Fukuda, M.; Tanigaki, M.

The magnetic moment of the proton drip-line nucleus {sup 9}C(I{sup {pi}}=3/2{sup -}, T{sub {1/2}}=126 ms) has been measured for the first time, using the {beta}-NMR detection technique with polarized radioactive beams. The measured value for the magnetic moment is {vert_bar} {mu}({sup 9}C) {vert_bar} = 1.3914{+-}0.0005 {mu}{sub N}. The deduced spin expectation value<{sigma}> of 1.44 is unusually larger than an other ones of even-odd nuclei.

Structure of 10 N in 9 C+p resonance scattering

DOE PAGES

Hooker, J.; Rogachev, G. V.; Goldberg, V. Z.; ...

2017-03-17

We studied the structure of exotic nucleus 10N using 9C+p resonance scattering. Two ℓ=0 resonances were found to be the lowest states in 10N. Furthermore, the ground state of 10N is unbound with respect to proton decay by 2.2(2) or 1.9(2) MeV depending on the 2 -or 1 -spin-parity assignment, and the first excited state is unbound by 2.8(2) MeV.

Nuclear structure and dynamics with density functional theory

NASA Astrophysics Data System (ADS)

Stetcu, Ionel

2015-10-01

Even in the absence of ab initio methods capable of tackling heavy nuclei without restrictions, one can obtain an ab initio description of ground-state properties by means of the density functional theory (DFT), and its extension to superfluid systems in its local variant, the superfluid local density approximation (SLDA). Information about the properties of excited states can be obtained in the same framework by using an extension to the time-dependent (TD) phenomena. Unlike other approaches in which the nuclear structure information is used as a separate input into reaction models, the TD approach treats on the same footing the nuclear structure and dynamics, and is well suited to provide more reliable description for a large number of processes involving heavy nuclei, from the nuclear response to electroweak probes, to nuclear reactions, such as neutron-induced reactions, or nuclear fusion and fission. Such processes, sometimes part of integrated nuclear systems, have important applications in astrophysics, energy production, global security, etc. In this talk, I will present the simulation of a simple reaction, that is the Coulomb excitation of a 238U nucleus, and discuss the application of the TD-DFT formalism to the description of induced fission. I gratefully acknowledge partial support of the U.S. Department of Energy through an Early Career Award of the LANL/LDRD Program.

Polarized photon scattering of 52Cr: Determining the parity of dipole states

NASA Astrophysics Data System (ADS)

Krishichayan, Fnu; Bhike, M.; Tornow, W.

2014-03-01

Observation of dipole states in nuclei are important because they provide information on various collective and single-particle nuclear excitation modes, e.g., pygmy dipole resonance (PDR) and spin-flip M1 resonance. The PDR has been extensively studied in the higher and medium mass region, whereas not much information is available around the low mass (A ~ 50) region where, apparently,the PDR starts to form. The present photoresponse of 52Cr has been investigated to test the evolution of the PDR in a nucleus with a small number of excess neutrons as well as to look for spin-flip M1 resonance excitation mode. Spin-1 states in 52Cr between 5.0 to 9.5 MeV excitation energy were excited by exploiting fully polarized photons using the (γ ,γ') nuclear resonance fluorescence technique, a completely model-independent electromagnetic method. The de-excitation γ-rays were detected using a HPGe array. The experiment was carried out using the HIGS facility at TUNL. Results of unambiguous parity determinations of dipole states in 52Cr will be presented.

Seven-quasiparticle bands in Ce139

NASA Astrophysics Data System (ADS)

Chanda, Somen; Bhattacharjee, Tumpa; Bhattacharyya, Sarmishtha; Mukherjee, Anjali; Basu, Swapan Kumar; Ragnarsson, I.; Bhowmik, R. K.; Muralithar, S.; Singh, R. P.; Ghugre, S. S.; Pramanik, U. Datta

2009-05-01

The high spin states in the Ce139 nucleus have been studied by in-beam γ-spectroscopic techniques using the reaction Te130(C12,3n)Ce139 at Ebeam=65 MeV. A gamma detector array, consisting of five Compton-suppressed Clover detectors was used for coincidence measurements. 15 new levels have been proposed and 28 new γ transitions have been assigned to Ce139 on the basis of γγ coincidence data. The level scheme of Ce139 has been extended above the known 70 ns (19)/(2)- isomer up to ~6.1 MeV in excitation energy and (35)/(2)ℏ in spin. The spin-parity assignments for most of the newly proposed levels have been made using the deduced Directional Correlation from Oriented states of nuclei (DCO ratio) and the Polarization Directional Correlation from Oriented states (PDCO ratio) for the de-exciting transitions. The observed level structure has been compared with a large basis shell model calculation and also with the predictions from cranked Nilsson-Strutinsky (CNS) calculations. A general consistency has been observed between these two different theoretical approaches.

In-beam γ -ray spectroscopy studies of medium-spin states in the odd-odd nucleus 186Re

NASA Astrophysics Data System (ADS)

Matters, D. A.; Kondev, F. G.; Aoi, N.; Ayyad, Y.; Byrne, A. P.; Carpenter, M. P.; Carroll, J. J.; Chiara, C. J.; Davidson, P. M.; Dracoulis, G. D.; Fang, Y. D.; Hoffman, C. R.; Hughes, R. O.; Ideguchi, E.; Janssens, R. V. F.; Kanaya, S.; Kay, B. P.; Kibédi, T.; Lane, G. J.; Lauritsen, T.; McClory, J. W.; Nieminen, P.; Noji, S.; Odahara, A.; Ong, H. J.; Stuchbery, A. E.; Tran, D. T.; Watanabe, H.; Wilson, A. N.; Yamamoto, Y.; Zhu, S.

2017-07-01

Excited states in 186Re with spins up to J =12 ℏ were investigated in two separate experiments using 186W(d ,2 n ) reactions at beam energies of 12.5 and 14.5 MeV. Two- and threefold γ -ray coincidence data were collected using the CAESAR and CAGRA spectrometers, respectively, each composed of Compton-suppressed high-purity germanium detectors. Analysis of the data revealed rotational bands built on several two-quasiparticle intrinsic states, including a long-lived Kπ=(8+) isomer. Configuration assignments were supported by an analysis of in-band properties, such as |gK-gR| values. The excitation energies of the observed intrinsic states were compared with results from multi-quasiparticle blocking calculations, based on the Lipkin-Nogami pairing approach, that included contributions from the residual proton-neutron interactions.

Model-independent analyses of dark-matter particle interactions

DOE PAGES

Anand, Nikhil; Fitzpatrick, A. Liam; Haxton, W. C.

2015-03-24

A model-independent treatment of dark-matter particle elastic scattering has been developed, yielding the most general interaction for WIMP-nucleon low-energy scattering, and the resulting amplitude has been embedded into the nucleus, taking into account the selection rules imposed by parity and time-reversal. One finds that, in contrast to the usual spin-independent/spin-dependent (SI/SD) formulation, the resulting cross section contains six independent nuclear response functions, three of which are associated with possible velocity-dependent interactions. We find that current experiments are four orders of magnitude more sensitive to derivative couplings than is apparent in the standard SI/SD treatment, which necessarily associated such interactions withmore » cross sections proportional to v 2 T ~ 10⁻⁶, where v T is the WIMP velocity relative to the center of mass of the nuclear target.« less

New nuclear structure data beyond 136Sn

NASA Astrophysics Data System (ADS)

Lozeva, Radomira

2018-05-01

Exotic nuclei beyond the 132Sn double shell-closure are influenced by both the Sn superfluity and the evolving collectivity only few nucleons away. Toward even more neutron-rich nuclei, especially at intermediate mass number, the interplay between single-particle and collective particle-hole excitations competes. In some cases with the extreme addition of neutrons also other effects as the formation of neutron skin, stabilization as sub-shell gaps or orbital crossings may be expected. The knowledge of nuclear ingredients is especially interesting beyond 132Sn and little is known on how the excitation modes develop with the addition of both protons and neutrons and for example systematic prompt and decay studies can be such very sensitive probe. Recently, we have approached this region of nuclei in several experimental measurements following 238U projectile fission on 9Be and n-induced fission on 241Pu and 235U. Consistent data analysis allows to access various spins and excitation energies and provide new input to theory. Examples from these studies on several nuclei in the A 140 region were presented during the conference together with the possible interpretation of the new data. Here, we will illustrate one example on 136I using two complementary data sets.

Spin coherence and 14N ESEEM effects of nitrogen-vacancy centers in diamond with X-band pulsed ESR

NASA Astrophysics Data System (ADS)

Rose, B. C.; Weis, C. D.; Tyryshkin, A. M.; Schenkel, T.; Lyon, S. A.

2017-02-01

Pulsed ESR experiments are reported for ensembles of negatively-charged nitrogen-vacancy centers (NV$^-$) in diamonds at X-band magnetic fields (280-400 mT) and low temperatures (2-70 K). The NV$^-$ centers in synthetic type IIb diamonds (nitrogen impurity concentration $<1$~ppm) are prepared with bulk concentrations of $2\\cdot 10^{13}$ cm$^{-3}$ to $4\\cdot 10^{14}$ cm$^{-3}$ by high-energy electron irradiation and subsequent annealing. We find that a proper post-radiation anneal (1000$^\\circ$C for 60 mins) is critically important to repair the radiation damage and to recover long electron spin coherence times for NV$^-$s. After the annealing, spin coherence times of T$_2 = 0.74$~ms at 5~K are achieved, being only limited by $^{13}$C nuclear spectral diffusion in natural abundance diamonds. At X-band magnetic fields, strong electron spin echo envelope modulation (ESEEM) is observed originating from the central $^{14}$N nucleus. The ESEEM spectral analysis allows for accurate determination of the $^{14}$N nuclear hypefine and quadrupole tensors. In addition, the ESEEM effects from two proximal $^{13}$C sites (second-nearest neighbor and fourth-nearest neighbor) are resolved and the respective $^{13}$C hyperfine coupling constants are extracted.

Application of relativistic mean field and effective field theory densities to scattering observables for Ca isotopes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bhuyan, M.; School of Physics, Sambalpur University, Jyotivihar, Burla 768 019; Panda, R. N.

In the framework of relativistic mean field (RMF) theory, we have calculated the density distribution of protons and neutrons for {sup 40,42,44,48}Ca with NL3 and G2 parameter sets. The microscopic proton-nucleus optical potentials for p+{sup 40,42,44,48}Ca systems are evaluated from the Dirac nucleon-nucleon scattering amplitude and the density of the target nucleus using relativistic-Love-Franey and McNeil-Ray-Wallace parametrizations. We have estimated the scattering observables, such as the elastic differential scattering cross section, analyzing power and the spin observables with the relativistic impulse approximation (RIA). The results have been compared with the experimental data for a few selective cases and we findmore » that the use of density as well as the scattering matrix parametrizations are crucial for the theoretical prediction.« less

Theory of Nuclear Quadrupole Interactions in the Chemical Ferromagnet p-Cl-Ph-CH-N=TEMPO

NASA Astrophysics Data System (ADS)

Briere, Tina M.; Jeong, Junho; Sahoo, N.; Das, T. P.; Ohira, S.; Nishiyama, K.; Nagamine, K.

2002-03-01

The study(Junho Jeong et al., Physica B 289-290, 132 (2000).) of the magnetic hyperfine properties of chemical ferromagnets provides valuable information about the electronic spin distributions in the individual molecules. Insights into the electronic charge distributions and their anisotropy can be obtained from electric quadrupole interactions for the different nuclei in these systems. For this purpose we have studied the nuclear quadrupole interactions(T. P. Das and E. L. Hahn "Nuclear Quadrupole Resonance Spectroscopy", Academic Press Inc., New York, 1958.) for the 14^N nuclei in the NO group and the bridge nitrogen, the 17^O nucleus in the NO group and the 35^Cl nucleus in the p-Cl-Ph-CH-N=TEMPO system both by itself and in the presence of trapped μ and Mu. Comparison will be made between our results and available experimental quadrupole coupling constant (e^2qQ) and asymmetry parameter (η) data.

Accumulation of linear mitochondrial DNA fragments in the nucleus shortens the chronological life span of yeast.

PubMed

Cheng, Xin; Ivessa, Andreas S

2012-10-01

Translocation of mitochondrial DNA (mtDNA) fragments to the nucleus and insertion of those fragments into nuclear DNA has been observed in several organisms ranging from yeast to plants and mammals. Disruption of specific nuclear genes by de novo insertions of mtDNA fragments has even been linked to the initiation of several human diseases. Recently, we demonstrated that baker's yeast strains with high rates of mtDNA fragments migrating to the nucleus (yme1-1 mutant) exhibit short chronological life spans (CLS). The yeast CLS is determined by the survival of non-dividing cell populations. Here, we show that lack of the non-homologous-end-joining enzyme DNA ligase IV (DNL4) can rescue the short CLS of the yme1-1 mutant. In fission yeast, DNA ligase IV has been shown to be required for the capture of mtDNA fragments during the repair of double-stranded DNA breaks in nuclear DNA. In further analyses using pulse field gel and 2D gel electrophoresis we demonstrate that linear mtDNA fragments with likely nuclear localization accumulate in the yme1-1 mutant. The accumulation of the linear mtDNA fragments in the yme1-1 mutant is suppressed when Dnl4 is absent. We propose that the linear nuclear mtDNA fragments accelerate the aging process in the yme1-1 mutant cells by possibly affecting nuclear processes including DNA replication, recombination, and repair as well as transcription of nuclear genes. We speculate further that Dnl4 protein has besides its function as a ligase also a role in DNA protection. Dnl4 protein may stabilize the linear mtDNA fragments in the nucleus by binding to their physical ends. In the absence of Dnl4 protein the linear fragments are therefore unprotected and possibly degraded by nuclear nucleases. Copyright © 2012 Elsevier GmbH. All rights reserved.

An Effective-Hamiltonian Approach to CH5+, Using Ideas from Atomic Spectroscopy

NASA Astrophysics Data System (ADS)

Hougen, Jon T.

2016-06-01

In this talk we present the first steps in the design of an effective Hamiltonian for the vibration-rotation energy levels of CH5+. Such a Hamiltonian would allow calculation of energy level patterns anywhere along the path travelled by a hypothetical CH5+ (or CD5+) molecule as it passes through various coupling cases, and might thus provide some hints for assigning the observed high-resolution spectra. The steps discussed here, which have not yet addressed computational problems, focus on mapping the vibration-rotation problem in CH5+ onto the five-electron problem in the boron atom, using ideas and mathematical machinery from Condon and Shortley's book on atomic spectroscopy. The mapping ideas are divided into: (i) a mapping of particles, (ii) a mapping of coordinates (i.e., mathematical degrees of freedom), and (iii) a mapping of quantum mechanical interaction terms. The various coupling cases along the path correspond conceptually to: (i) the analog of a free-rotor limit, where the H atoms see the central C atom but do not see each other, (ii) the low-barrier and high-barrier tunneling regimes, and (iii) the rigid-molecule limit, where the H atoms remain locked in some fixed molecular geometry. Since the mappings considered here often involve significant changes in mathematics, a number of interesting qualitative changes occur in the basic ideas when passing from B to CH5+, particularly in discussions of: (i) antisymmetrization and symmetrization ideas, (ii) n,l,ml,ms or n,l,j,mj quantum numbers, and (iii) Russell-Saunders computations and energy level patterns. Some of the mappings from B to CH5+ to be discussed are as follows. Particles: the atomic nucleus is replaced by the C atom, the electrons are replaced by protons, and the empty space between particles is replaced by an "electron soup." Coordinates: the radial coordinates of the electrons map onto the five local C-H stretching modes, the angular coordinates of the electrons map onto three rotational degrees of freedom and seven bending vibrational degrees of freedom. The half-integral electron spins map onto half-integral proton spins or onto integral deuterium spins (for CD5+). Interactions: the Coulomb attraction between nucleus and electrons maps onto a Morse-oscillator C-H stretching potential, spin-orbit interaction maps onto proton-spin-overall-rotation interaction, and Coulomb repulsion between electrons maps onto some kind of proton repulsion that leads to the equilibrium geometry.

Nuclear magnetic resonance shielding constants and chemical shifts in linear 199Hg compounds: a comparison of three relativistic computational methods.

PubMed

Arcisauskaite, Vaida; Melo, Juan I; Hemmingsen, Lars; Sauer, Stephan P A

2011-07-28

We investigate the importance of relativistic effects on NMR shielding constants and chemical shifts of linear HgL(2) (L = Cl, Br, I, CH(3)) compounds using three different relativistic methods: the fully relativistic four-component approach and the two-component approximations, linear response elimination of small component (LR-ESC) and zeroth-order regular approximation (ZORA). LR-ESC reproduces successfully the four-component results for the C shielding constant in Hg(CH(3))(2) within 6 ppm, but fails to reproduce the Hg shielding constants and chemical shifts. The latter is mainly due to an underestimation of the change in spin-orbit contribution. Even though ZORA underestimates the absolute Hg NMR shielding constants by ∼2100 ppm, the differences between Hg chemical shift values obtained using ZORA and the four-component approach without spin-density contribution to the exchange-correlation (XC) kernel are less than 60 ppm for all compounds using three different functionals, BP86, B3LYP, and PBE0. However, larger deviations (up to 366 ppm) occur for Hg chemical shifts in HgBr(2) and HgI(2) when ZORA results are compared with four-component calculations with non-collinear spin-density contribution to the XC kernel. For the ZORA calculations it is necessary to use large basis sets (QZ4P) and the TZ2P basis set may give errors of ∼500 ppm for the Hg chemical shifts, despite deceivingly good agreement with experimental data. A Gaussian nucleus model for the Coulomb potential reduces the Hg shielding constants by ∼100-500 ppm and the Hg chemical shifts by 1-143 ppm compared to the point nucleus model depending on the atomic number Z of the coordinating atom and the level of theory. The effect on the shielding constants of the lighter nuclei (C, Cl, Br, I) is, however, negligible. © 2011 American Institute of Physics

Proton Resonance Spectroscopy in CALCIUM-40.

NASA Astrophysics Data System (ADS)

Warthen, Barry Joseph

1987-09-01

The differential cross sections for the ^{39}K(p,p_{ rm o})^{39}K and ^{39}K(p,alpha_ {rm o})^{36}Ar reactions have been measured for E_{ rm p} = 1.90 to 4.02 MeV at laboratory angles theta = 90^ circ, 108^circ, 150^circ and 165^ circ. Data were taken with the Triangle Universities Nuclear Laboratory (TUNL) KN Van de Graaff accelerator and the associated high resolution system. The targets consisted of 1-2 mug/cm^2 of potassium carbonate (K_2CO _3), enriched to 99.97% ^{39}K, evaporated onto gold coated carbon backings. Excitation functions were measured in proton energy steps varying from 100 to 400 eV. The energy region studied corresponds to an excitation energy range in the ^{40}Ca nucleus of E_{rm x} = 10.2 to 12.3 MeV. A multi-level multi-channel R-matrix based computer code was used to fit the experimental excitation functions. Resonance parameters obtained include resonance energy, spin, parity, partial widths, and channel spin and orbital angular momentum mixing ratios. Of the 248 resonances observed in the proton channel, 148 were also observed in the alpha channel. A fit to the observed level density yielded a nuclear temperature of 1.5 MeV. The data were compared with predictions of statistical theories of energy levels for both level spacing and reduced width distributions. The alpha reduced widths agree with the Porter-Thomas distribution and suggest that only 5-10% of the states with alpha widths were not observed. The summed strength in each of the alpha channels represents a significant fraction of the Wigner limit for these channels. The proton channels, on the other hand, generally have much smaller fractions. The two proton s-wave strength functions are equal and thus show no evidence for spin-exchange forces in the nucleon-nucleus interaction.

Free radical generation by non-equilibrium atmospheric pressure plasma in alcohol-water mixtures: an EPR-spin trapping study

NASA Astrophysics Data System (ADS)

Uchiyama, Hidefumi; Ishikawa, Kenji; Zhao, Qing-Li; Andocs, Gabor; Nojima, Nobuyuki; Takeda, Keigo; Krishna, Murali C.; Ishijima, Tatsuo; Matsuya, Yuji; Hori, Masaru; Noguchi, Kyo; Kondo, Takashi

2018-03-01

Free radical species in aqueous solution—various alcohol-water reaction mixtures—by exposure to non-equilibrium cold atmospheric pressure Ar plasma (CAP), were monitored using electron paramagnetic resonance spin-trapping techniques with 3, 5-dibromo-4-nitrosobenzene sulfonate as a water soluble nitroso spin trap. The major radical species were formed by H-abstraction from alcohol molecules due to ·OH radicals. In the ethanol-water mixture ·CH2CH2OH produced by H abstraction from CH3 group of the ethanol and ·CH3 radicals were detected. The latter was due to the decomposition of unstable CH3·CHOH to form the ·CH3 radicals and the stable formaldehyde by C-C bond fission. These intermediates are similar to those observed by reaction with ·OH radicals generation in the H2O2-UV photolysis of the reaction mixtures. The evidence of ·CH3 radical formation in the pyrolytic decomposition of the reaction mixtures by exposure to ultrasound or in methane irradiated with microwave plasma have been reported previously. However, the pyrolytic ·CH3 radicals were not found in both plasma and H2O2-UV photolysis condition. These results suggests that free radicals produced by Ar-CAP are most likely due to the reaction between abundant ·OH radicals and alcohol molecules.

Pre-compound emission in low-energy heavy-ion interactions

NASA Astrophysics Data System (ADS)

Sharma, Manoj Kumar; Shuaib, Mohd.; Sharma, Vijay R.; Yadav, Abhishek; Singh, Pushpendra P.; Singh, Devendra P.; Unnati; Singh, B. P.; Prasad, R.

2017-11-01

Recent experimental studies have shown the presence of pre-compound emission component in heavy ion reactions at low projectile energy ranging from 4 to 7 MeV/nucleons. In earlier measurements strength of the pre-compound component has been estimated from the difference in forward-backward distributions of emitted particles. Present measurement is a part of an ongoing program on the study of reaction dynamics of heavy ion interactions at low energies aimed at investigating the effect of momentum transfer in compound, precompound, complete and incomplete fusion processes in heavy ion reactions. In the present work on the basis of momentum transfer the measurement of the recoil range distributions of heavy residues has been used to decipher the components of compound and pre-compound emission processes in the fusion of 16O projectile with 159Tb and 169Tm targets. The analysis of recoil range distribution measurements show two distinct linear momentum transfer components corresponding to pre-compound and compound nucleus processes are involved. In order to obtain the mean input angular momentum associated with compound and pre-compound emission processes, an online measurement of the spin distributions of the residues has been performed. The analysis of spin distribution indicate that the mean input angular momentum associated with pre-compound products is found to be relatively lower than that associated with compound nucleus process. The pre-compound components obtained from the present analysis are consistent with those obtained from the analysis of excitation functions.

Prospects for dark matter detection with inelastic transitions of xenon

DOE Office of Scientific and Technical Information (OSTI.GOV)

McCabe, Christopher

2016-05-16

Dark matter can scatter and excite a nucleus to a low-lying excitation in a direct detection experiment. This signature is distinct from the canonical elastic scattering signal because the inelastic signal also contains the energy deposited from the subsequent prompt de-excitation of the nucleus. A measurement of the elastic and inelastic signal will allow a single experiment to distinguish between a spin-independent and spin-dependent interaction. For the first time, we characterise the inelastic signal for two-phase xenon detectors in which dark matter inelastically scatters off the {sup 129}Xe or {sup 131}Xe isotope. We do this by implementing a realistic simulationmore » of a typical tonne-scale two-phase xenon detector and by carefully estimating the relevant background signals. With our detector simulation, we explore whether the inelastic signal from the axial-vector interaction is detectable with upcoming tonne-scale detectors. We find that two-phase detectors allow for some discrimination between signal and background so that it is possible to detect dark matter that inelastically scatters off either the {sup 129}Xe or {sup 131}Xe isotope for dark matter particles that are heavier than approximately 100 GeV. If, after two years of data, the XENON1T search for elastic scattering nuclei finds no evidence for dark matter, the possibility of ever detecting an inelastic signal from the axial-vector interaction will be almost entirely excluded.« less

Feasibility studies towards future self-sufficient supply of the 99Mo-99mTc isotopes with Japanese accelerators

PubMed Central

NAKAI, Kozi; TAKAHASHI, Naruto; HATAZAWA, Jun; SHINOHARA, Atsushi; HAYASHI, Yoshihiko; IKEDA, Hayato; KANAI, Yasukazu; WATABE, Tadashi; FUKUDA, Mitsuhiro; HATANAKA, Kichiji

2014-01-01

In order to establish a self-sufficient supply of 99mTc, we studied feasibilities to produce its parent nucleus, 99Mo, using Japanese accelerators. The daughter nucleus, 99mTc, is indispensable for medical diagnosis. 99Mo has so far been imported from abroad, which is separated from fission products generated in nuclear reactors using enriched 235U fuel. We investigated 99mTc production possibilities based on the following three scenarios: (1) 99Mo production by the (n, 2n) reaction by spallation neutrons at the J-PARC injector, LINAC; (2) 99Mo production by the (p, pn) reaction at Ep = 50–80 MeV proton at the RCNP cyclotron; (3) 99mTc direct production with a 20 MeV proton beam from the PET cyclotron. Among these three scenarios, scenario (1) is for a scheme on a global scale, scenario (2) works in a local area, and both cases take a long time for negotiations. Scenario (3) is attractive because we can use nearly 50 PET cyclotrons in Japan for 99mTc production. We here consider both the advantages and disadvantages among the three scenarios by taking account of the Japanese accelerator situation. PMID:25504230

Monopole-driven shell evolution below the doubly magic nucleus 132Sn explored with the long-lived isomer in 126Pd.

PubMed

Watanabe, H; Lorusso, G; Nishimura, S; Otsuka, T; Ogawa, K; Xu, Z Y; Sumikama, T; Söderström, P-A; Doornenbal, P; Li, Z; Browne, F; Gey, G; Jung, H S; Taprogge, J; Vajta, Zs; Wu, J; Yagi, A; Baba, H; Benzoni, G; Chae, K Y; Crespi, F C L; Fukuda, N; Gernhäuser, R; Inabe, N; Isobe, T; Jungclaus, A; Kameda, D; Kim, G D; Kim, Y K; Kojouharov, I; Kondev, F G; Kubo, T; Kurz, N; Kwon, Y K; Lane, G J; Moon, C-B; Montaner-Pizá, A; Moschner, K; Naqvi, F; Niikura, M; Nishibata, H; Nishimura, D; Odahara, A; Orlandi, R; Patel, Z; Podolyák, Zs; Sakurai, H; Schaffner, H; Simpson, G S; Steiger, K; Suzuki, H; Takeda, H; Wendt, A; Yoshinaga, K

2014-07-25

A new isomer with a half-life of 23.0(8) ms has been identified at 2406 keV in (126)Pd and is proposed to have a spin and parity of 10(+) with a maximally aligned configuration comprising two neutron holes in the 1h(11/2) orbit. In addition to an internal-decay branch through a hindered electric octupole transition, β decay from the long-lived isomer was observed to populate excited states at high spins in (126)Ag. The smaller energy difference between the 10(+) and 7(-) isomers in (126)Pd than in the heavier N=80 isotones can be interpreted as being ascribed to the monopole shift of the 1h(11/2) neutron orbit. The effects of the monopole interaction on the evolution of single-neutron energies below (132)Sn are discussed in terms of the central and tensor forces.

A new phenomenological /τ-/α interaction

NASA Astrophysics Data System (ADS)

Heiberg-Andersen, H.; Mackintosh, R. S.; Vaagen, J. S.

2003-01-01

We present a potential model, with distinctive features, reproducing angular distributions and analyzing power data for τ- α scattering from 20 to 30 MeV τ energy with regular variation of the parameters. The distinctive features are: (1) a spin-orbit term which incorporates the influence of central depression in the α nucleus, and, (2) central terms which are strongly parity dependent. The parity dependence of the real central term is such that the odd-parity component has both a greater rms radius and greater volume integral than the even-parity component. These parity dependence characteristics had been predicted by the inversion of the RGM S-matrix. Our result supports a considerable contribution from three-nucleon exchange processes. The predicted 1/2 - level of 7Be is shifted 3 MeV relative to a previous one-level R-matrix formula fit, and depends strongly on the geometry of the spin-orbit potential.

In-beam γ -ray spectroscopy studies of medium-spin states in the odd-odd nucleus Re 186

DOE Office of Scientific and Technical Information (OSTI.GOV)

Matters, D. A.; Kondev, F. G.; Aoi, N.

2017-07-01

Excited states in 186Re with spins up to J = 12~ were investigated in two separate experiments using 186W(d, 2n) reactions at beam energies of 12.5 MeV and 14.5 MeV. Two- and three-fold γ-ray coincidence data were collected using the CAESAR and CAGRA spectrometers, respectively, each composed of Compton-suppressed HpGe detectors. Analysis of the data revealed rotational bands built on several two-quasiparticle intrinsic states, including a long-lived Kπ = (8+) isomer. Configuration assignments were supported by an analysis of in-band properties, such as |gK - gR| values. The excitation energies of the observed intrinsic states were compared with results frommore » multiquasiparticle blocking calculations, based on the Lipkin-Nogami pairing approach, that included contributions from the residual proton-neutron interactions.« less

Physics opportunities with a fixed target experiment at the LHC (AFTER@LHC)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hadjidakis, Cynthia; Anselmino, Mauro; Arnaldi, R.

By extracting the beam with a bent crystal or by using an internal gas target, the multi-TeV proton and lead LHC beams allow one to perform the most energetic fixed-target experiments (AFTER@LHC) and to study p+p and p+A collisions at \\sqrt{s_NN}=115 GeV and Pb+p and Pb+A collisions at \\sqrt{s_NN}=72 GeV. Such studies would address open questions in the domain of the nucleon and nucleus partonic structure at high-x, quark-gluon plasma and, by using longitudinally or transversally polarised targets, spin physics. In this paper, we discuss the physics opportunities of a fixed-target experiment at the LHC and we report on themore » possible technical implementations of a high-luminosity experiment. We finally present feasibility studies for Drell-Yan, open heavy-flavour and quarkonium production, with an emphasis on high-x and spin physics.« less

Fission and quasifission of composite systems with Z =108 -120 : Transition from heavy-ion reactions involving S and Ca to Ti and Ni ions

NASA Astrophysics Data System (ADS)

Kozulin, E. M.; Knyazheva, G. N.; Novikov, K. V.; Itkis, I. M.; Itkis, M. G.; Dmitriev, S. N.; Oganessian, Yu. Ts.; Bogachev, A. A.; Kozulina, N. I.; Harca, I.; Trzaska, W. H.; Ghosh, T. K.

2016-11-01

Background: Suppression of compound nucleus formation in the reactions with heavy ions by a quasifission process in dependence on the reaction entrance channel. Purpose: Investigation of fission and quasifission processes in the reactions 36S,48Ca,48Ti , and 64Ni+238U at energies around the Coulomb barrier. Methods: Mass-energy distributions of fissionlike fragments formed in the reaction 48Ti+238U at energies of 247, 258, and 271 MeV have been measured using the double-arm time-of-flight spectrometer CORSET at the U400 cyclotron of the Flerov Laboratory of Nuclear Reactions and compared with mass-energy distributions for the reactions 36S,48Ca,64Ni+238U . Results: The most probable fragment masses as well as total kinetic energies and their dispersions in dependence on the interaction energies have been investigated for asymmetric and symmetric fragments for the studied reactions. The fusion probabilities have been deduced from the analysis of mass-energy distributions. Conclusion: The estimated fusion probability for the reactions S, Ca, Ti, and Ni ions with actinide nuclei shows that it depends exponentially on the mean fissility parameter of the system. For the reactions with actinide nuclei leading to the formation of superheavy elements the fusion probabilities are of several orders of magnitude higher than in the case of cold fusion reactions.

Table of superdeformed nuclear bands and fission isomers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Firestone, R.B.; Singh, B.

A minimum in the second potential well of deformed nuclei was predicted and the associated shell gaps are illustrated in the harmonic oscillator potential shell energy surface calculations shown in this report. A strong superdeformed minimum in {sup 152}Dy was predicted for {beta}{sub 2}-0.65. Subsequently, a discrete set of {gamma}-ray transitions in {sup 152}DY was observed and, assigned to the predicted superdeformed band. Extensive research at several laboratories has since focused on searching for other mass regions of large deformation. A new generation of {gamma}-ray detector arrays is already producing a wealth of information about the mechanisms for feeding andmore » deexciting superdeformed bands. These bands have been found in three distinct regions near A=l30, 150, and 190. This research extends upon previous work in the actinide region near A=240 where fission isomers were identified and also associated with the second potential well. Quadrupole moment measurements for selected cases in each mass region are consistent with assigning the bands to excitations in the second local minimum. As part of our committment to maintain nuclear structure data as current as possible in the Evaluated Nuclear Structure Reference File (ENSDF) and the Table of Isotopes, we have updated the information on superdeformed nuclear bands. As of April 1994, we have complied data from 86 superdeformed bands and 46 fission isomers identified in 73 nuclides for this report. For each nuclide there is a complete level table listing both normal and superdeformed band assignments; level energy, spin, parity, half-life, magneto moments, decay branchings; and the energies, final levels, relative intensities, multipolarities, and mixing ratios for transitions deexciting each level. Mass excess, decay energies, and proton and neutron separation energies are also provided from the evaluation of Audi and Wapstra.« less

Elastic and inelastic scattering for the 10B+58Ni system at near-barrier energies

NASA Astrophysics Data System (ADS)

Scarduelli, V.; Crema, E.; Guimarães, V.; Abriola, D.; Arazi, A.; de Barbará, E.; Capurro, O. A.; Cardona, M. A.; Gallardo, J.; Hojman, D.; Martí, G. V.; Pacheco, A. J.; Rodrígues, D.; Yang, Y. Y.; Deshmukh, N. N.; Paes, B.; Lubian, J.; Mendes Junior, D. R.; Morcelle, V.; Monteiro, D. S.

2017-11-01

Full angular distributions of the 10B elastically and inelastically scattered by 58Ni have been measured at different energies around the Coulomb barrier. The elastic and inelastic scattering of 10B on a medium mass target has been measured for the first time. The obtained angular distributions have been analyzed in terms of large-scale coupled reaction channel calculations, where several inelastic transitions of the projectile and the target, as well as the most relevant one- and two-step transfer reactions have been included in the coupling matrix. The roles of the spin reorientation, the spin-orbit interaction, and the large ground-state deformation of the 10B, in the reaction mechanism, were also investigated. The real part of the interaction potential between projectile and target was represented by a parameter-free double-folding potential, whereas no imaginary potential at the surface was considered. In this sense, the theoretical calculations were parameter free and their results were compared to experimental data to investigate the relative importance of the different reaction channels. A striking influence of the ground-state spin reorientation of the 10B nucleus was found, while all transfer reactions investigated had a minimum contribution to the dynamics of the system. Finally, the large static deformation of the 10B and the spin-orbit coupling can also play an important role in the system studied.

Summary report on UO 2 thermal conductivity model refinement and assessment studies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Xiang-Yang; Cooper, Michael William Donald; Mcclellan, Kenneth James

Uranium dioxide (UO 2) is the most commonly used fuel in light water nuclear reactors and thermal conductivity controls the removal of heat produced by fission, therefore, governing fuel temperature during normal and accident conditions. The use of fuel performance codes by the industry to predict operational behavior is widespread. A primary source of uncertainty in these codes is thermal conductivity, and optimized fuel utilization may be possible if existing empirical models were replaced with models that incorporate explicit thermal conductivity degradation mechanisms during fuel burn-up. This approach is able to represent the degradation of thermal conductivity due to eachmore » individual defect type, rather than the overall burn-up measure typically used which is not an accurate representation of the chemical or microstructure state of the fuel that actually governs thermal conductivity and other properties. To generate a mechanistic thermal conductivity model, molecular dynamics (MD) simulations of UO 2 thermal conductivity including representative uranium and oxygen defects and fission products are carried out. These calculations employ a standard Buckingham type interatomic potential and a potential that combines the many-body embedded atom method potential with Morse-Buckingham pair potentials. Potential parameters for UO 2+x and ZrO 2 are developed for the latter potential. Physical insights from the resonant phonon-spin scattering mechanism due to spins on the magnetic uranium ions have been introduced into the treatment of the MD results, with the corresponding relaxation time derived from existing experimental data. High defect scattering is predicted for Xe atoms compared to that of La and Zr ions. Uranium defects reduce the thermal conductivity more than oxygen defects. For each defect and fission product, scattering parameters are derived for application in both a Callaway model and the corresponding high-temperature model typically used in fuel performance codes. The model is validated by comparison to low-temperature experimental measurements on single crystal hyper-stoichiometric UO 2+x samples and high-temperature literature data. Ongoing works include investigation of the effect of phase separation to UO 2+U 4O 9 on the low temperature thermal conductivity of UO 2+x, and modeling of thermal conductivity using the Green-Kubo method. Ultimately, this work will enable more accurate fuel performance simulations as well as extension to new fuel types and operating conditions, all of which improve the fuel economics of nuclear energy and maintain high fuel reliability and safety.« less

Gemini and Keck Observations of Slowly Rotating, Bilobate Active Asteroid (300163)

NASA Astrophysics Data System (ADS)

Waniak, Waclaw; Drahus, Michal

2016-10-01

One of the most puzzling questions regarding Active Asteroids is the mechanism of their activation. While some Active Asteroids show protracted and often recurrent mass loss, consistent with seasonal ice sublimation, some other eject dust impulsively as a result of a catastrophic disruption (e.g. Jewitt et al. 2015, Asteroids IV, 221). It has been suggested that ice can be excavated from the cold near-surface interior by an impact (Hsieh & Jewitt 2006, Science 312, 561) or, for small objects susceptible to YORP torques, by near-critical spin rate (Sheppard & Trujillo 2014, AJ 149, 44). But impact and rapid spin can also cause a catastrophic disruption (e.g. Jewitt et al. 2015, Asteroids IV, 221). It therefore becomes apparent that the different types of mass loss observed in Active Asteroids can be best classified and understood based on the nucleus spin rates (Drahus et al. 2015, ApJL 802, L8), but unfortunately the rotation periods have been measured for a very limited number of these objects. With this in mind we have initiated a survey of light curves of small Active Asteroids on the largest ground-based optical telescopes. Here we present the results for (300163), also known as 288P and 2006 VW139, which is a small 2.6-km sized asteroid that exhibited a comet-like activity over 100 days in the second half of 2011 (Hsieh et al. 2012, ApJL 748, L15; Licandro et al. 2013, A&A 550, A17; Agarwal et al. 2016, AJ 151, 12). Using Keck/DEIMOS and Gemini/GMOS-S working in tandem on UT 2015 May 21-22 we have detected an inactive nucleus and measured a complete, dense, high-S/N rotational light curve. The light curve has a double-peaked period of 16 hours, an amplitude of 0.4 mag, and moderately narrow minima suggesting a bilobate or contact-binary shape. The long rotation period clearly demonstrates a non-rotational origin of activity of this object, consistent with an impact. Furthermore, among the five small Active Asteroids with known rotation periods (300163) is only the second object with a confirmed slow spin rate, the other three rotating rapidly, near the limit of rotational stability. This suggests that rotation- and impact-driven origin of activity can be comparably common among small asteroids.

Astrophysical relevance of the low-energy dipole strength of 206Pb

NASA Astrophysics Data System (ADS)

Tonchev, A. P.; Tsoneva, N.; Goriely, S.; Bhatia, C.; Arnold, C. W.; Hammond, S. L.; Kelley, J. H.; Kwan, E.; Lenske, H.; Piekarewicz, J.; Raut, R.; Rusev, G.; Shizuma, T.; Tornow, W.

2018-05-01

The dipole strength of 206Pb was studied below the neutron separation energy using photon scattering experiments at the HIGS facility. Utilizing the technique of nuclear resonance fluorescence with 100% linearly-polarized photon beams, the spins, parities, branching ratios and decay widths of excited states in 206Pb from 4.9 - 8.1 MeV have been measured. The new experimental information is used to reliably predict the neutron capture cross section of 205Pb, an important branch point nucleus along the s-process path of nucleosynthesis.

Analysis and interpretation of CCD data on P/Halley and physical parameters and activity status of cometary nuclei at large heliocentric distance

NASA Technical Reports Server (NTRS)

Belton, Michael J. S.; Mueller, Beatrice

1991-01-01

The scientific objectives were as follows: (1) to construct a well sampled photometric time series of comet Halley extending to large heliocentric distances both post and pre-perihelion passage and derive a precise ephemeris for the nuclear spin so that the physical and chemical characteristics of individual regions of activity on the nucleus can be determined; and (2) to extend the techniques in the study of Comet Halley to the study of other cometary nuclei and to obtain new observational data.

Magnetic dipole excitations of 50Cr

NASA Astrophysics Data System (ADS)

Pai, H.; Beck, T.; Beller, J.; Beyer, R.; Bhike, M.; Derya, V.; Gayer, U.; Isaak, J.; Krishichayan, Kvasil, J.; Löher, B.; Nesterenko, V. O.; Pietralla, N.; Martínez-Pinedo, G.; Mertes, L.; Ponomarev, V. Yu.; Reinhard, P.-G.; Repko, A.; Ries, P. C.; Romig, C.; Savran, D.; Schwengner, R.; Tornow, W.; Werner, V.; Wilhelmy, J.; Zilges, A.; Zweidinger, M.

2016-01-01

The low-lying M 1 strength of the open-shell nucleus 50Cr has been studied with the method of nuclear resonance fluorescence up to 9.7 MeV using bremsstrahlung at the superconducting Darmstadt linear electron accelerator S-DALINAC and Compton backscattered photons at the High Intensity γ -ray Source (HI γ S ) facility between 6 and 9.7 MeV of the initial photon energy. Fifteen 1+ states have been observed between 3.6 and 9.7 MeV. Following our analysis the lowest 1+ state at 3.6 MeV can be considered as an isovector orbital mode with some spin admixture. The obtained results generally match the estimations and trends typical for the scissors-like mode. Detailed calculations within the Skyrme quasiparticle random-phase-approximation method and the large-scale shell model justify our conclusions. The calculated distributions of the orbital current for the lowest 1+-state suggest the schematic view of Lipparini and Stringari (isovector rotation-like oscillations inside the rigid surface) rather than the scissors-like picture of Lo Iudice and Palumbo. The spin M 1 resonance is shown to be mainly generated by spin-flip transitions between the orbitals of the f p shell.

NMR study of heavy fermion compound EuNi2P2

NASA Astrophysics Data System (ADS)

Magishi, K.; Watanabe, R.; Hisada, A.; Saito, T.; Koyama, K.; Fujiwara, T.

2015-03-01

We report the results of 31P-nuclear magnetic resonance (NMR) measurements on heavy fermion compound EuNi2P2 in order to investigate the magnetic properties at low temperatures from a microscopic view point. The Knight shift has a negative value in an entire temperature range, and the absolute value increases with decreasing temperature but exhibits a broad maximum around 40 K, which is similar to the behavior of the magnetic susceptibility. Also, the nuclear spin-lattice relaxation rate 1/T1 is almost constant at high temperatures above 200 K, which is reminiscent of the relaxation mechanism dominated by the interaction of the 31P nucleus with fluctuating Eu-4f moments. Below 200 K, 1/T1 gradually decreases on cooling due to the change of the valence in the Eu ion. At low temperatures, 1/T1 does not obey the Korringa relation, in contrast to typical heavy fermion compounds. The nuclear spin-spin relaxation rate 1/T2 shows the similar behavior as 1/T1 at high temperatures. But, below 50 K, 1/T2 increases upon cooling due to the development of the magnetic excitation.

An improved numerical method to compute neutron/gamma deexcitation cascades starting from a high spin state

DOE PAGES

Regnier, D.; Litaize, O.; Serot, O.

2015-12-23

Numerous nuclear processes involve the deexcitation of a compound nucleus through the emission of several neutrons, gamma-rays and/or conversion electrons. The characteristics of such a deexcitation are commonly derived from a total statistical framework often called “Hauser–Feshbach” method. In this work, we highlight a numerical limitation of this kind of method in the case of the deexcitation of a high spin initial state. To circumvent this issue, an improved technique called the Fluctuating Structure Properties (FSP) method is presented. Two FSP algorithms are derived and benchmarked on the calculation of the total radiative width for a thermal neutron capture onmore » 238U. We compare the standard method with these FSP algorithms for the prediction of particle multiplicities in the deexcitation of a high spin level of 143Ba. The gamma multiplicity turns out to be very sensitive to the numerical method. The bias between the two techniques can reach 1.5 γγ/cascade. Lastly, the uncertainty of these calculations coming from the lack of knowledge on nuclear structure is estimated via the FSP method.« less

Seven-quasiparticle bands in {sup 139}Ce

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chanda, Somen; Bhattacharjee, Tumpa; Bhattacharyya, Sarmishtha

2009-05-15

The high spin states in the {sup 139}Ce nucleus have been studied by in-beam {gamma}-spectroscopic techniques using the reaction {sup 130}Te({sup 12}C,3n){sup 139}Ce at E{sub beam}=65 MeV. A gamma detector array, consisting of five Compton-suppressed Clover detectors was used for coincidence measurements. 15 new levels have been proposed and 28 new {gamma} transitions have been assigned to {sup 139}Ce on the basis of {gamma}{gamma} coincidence data. The level scheme of {sup 139}Ce has been extended above the known 70 ns (19/2){sup -} isomer up to {approx}6.1 MeV in excitation energy and (35/2)({Dirac_h}/2{pi}) in spin. The spin-parity assignments for most ofmore » the newly proposed levels have been made using the deduced Directional Correlation from Oriented states of nuclei (DCO ratio) and the Polarization Directional Correlation from Oriented states (PDCO ratio) for the de-exciting transitions. The observed level structure has been compared with a large basis shell model calculation and also with the predictions from cranked Nilsson-Strutinsky (CNS) calculations. A general consistency has been observed between these two different theoretical approaches.« less

Artificial tektites: an experimental technique for capturing the shapes of spinning drops

NASA Astrophysics Data System (ADS)

Baldwin, Kyle A.; Butler, Samuel L.; Hill, Richard J. A.

2015-01-01

Determining the shapes of a rotating liquid droplet bound by surface tension is an archetypal problem in the study of the equilibrium shapes of a spinning and charged droplet, a problem that unites models of the stability of the atomic nucleus with the shapes of astronomical-scale, gravitationally-bound masses. The shapes of highly deformed droplets and their stability must be calculated numerically. Although the accuracy of such models has increased with the use of progressively more sophisticated computational techniques and increases in computing power, direct experimental verification is still lacking. Here we present an experimental technique for making wax models of these shapes using diamagnetic levitation. The wax models resemble splash-form tektites, glassy stones formed from molten rock ejected from asteroid impacts. Many tektites have elongated or `dumb-bell' shapes due to their rotation mid-flight before solidification, just as we observe here. Measurements of the dimensions of our wax `artificial tektites' show good agreement with equilibrium shapes calculated by our numerical model, and with previous models. These wax models provide the first direct experimental validation for numerical models of the equilibrium shapes of spinning droplets, of importance to fundamental physics and also to studies of tektite formation.

Asteroid clusters similar to asteroid pairs

NASA Astrophysics Data System (ADS)

Pravec, Petr; Vokrouhlicky, David; Fatka, Petr; Kusnirák, Peter; Hornoch, Kamil; Galád, Adrián

2016-10-01

We study five small, tight and young clusters of asteroids. They are placed around following largest (primary) bodies: (11842) Kap'bos, (14627) Emilkowalski, (16598) 1992 YC2, (21509) Lucascavin and (39991) 1998 HR37. Each cluster has 2-4 secondaries that are tightly clustered around the primary body, with distance in the 5-dimensional space of mean orbital elements mostly within 10 m/s, and always < 23 m/s. Backward orbital integrations indicate that they formed between 105 and 106 yr ago. In the P1-q space, where P1 is the primary's spin period and q = Σ Mj/M1 is the total secondary-to-primary mass ratio, the clusters lie in the same range as asteroid pairs formed by rotational fission. We have extended the model of a proto-system separation after rotational fission by Pravec et al. (2010) for application to systems with more than one secondary and found a perfect match for the five tight clusters. We find these clusters to be similar to asteroid pairs and we suggest that they are "extended pairs", having 2-4 escaped secondaries rather than just one secondary as in the case of an asteroid pair. We compare them to six young mini-families (1270) Datura, (2384) Schulhof, (3152) Jones, (6825) Irvine, (10321) Rampo and (20674) 1999 VT1. These mini-families have similar ages, but they have a higher number of members and/or they show a significantly larger spread in the mean orbital elements (dmean on an order of tens m/s) than the five tight clusters. In the P1-q space, all but one of the mini-families lie in the same range as asteroid pairs and the tight clusters; the exception is the mini-family of (3152) Jones which appears to be a collisional family. A possibility that the other five mini-families were also formed by rotational fission as we suggest for the tight clusters ("extended asteroid pairs") is being explored.Reference:Pravec, P., et al. Formation of asteroid pairs by rotational fission. Nature 466, 1085-1088.

Observation of γ-vibrations and alignments built on non-ground-state configurations in ¹⁵⁶Dy

DOE PAGES

Zhu, C. -H.; Hartley, D. J.; Riedinger, L. L.; ...

2015-03-26

The exact nature of the lowest K π=2⁺ rotational bands in all deformed nuclei remains obscure. Traditionally they are assumed to be collective vibrations of the nuclear shape in the γ degree of freedom perpendicular to the nuclear symmetry axis. Very few such γ-bands have been traced past the usual back-bending rotational alignments of high-j nucleons. We have investigated the structure of positive-parity bands in the N=90 nucleus ¹⁵⁶Dy, using the ¹⁴⁸Nd(¹²C,4n)¹⁵⁶Dy reaction at 65 MeV, observing the resulting γ-ray transitions with the Gammasphere array. The even- and odd-spin members of the π=2⁺ γ-band are observed to 32⁺ and 31⁺more » respectively. This rotational band faithfully tracks the ground-state configuration to the highest spins. The members of a possible γ-vibration built on the aligned yrast S-band are observed to spins 28⁺ and 27⁺. An even-spin positive-parity band, observed to spin 24⁺, is a candidate for an aligned S-band built on the seniority-zero configuration of the 0₂⁺ state at 676 keV. As a result, the crossing of this band with the 0₂⁺ band is at hw c = 0.28(1) MeV and is consistent with the configuration of the 0₂⁺ band not producing any blocking of the monopole pairing.« less

Measurements of the Double-Spin Asymmetry A 1 on Helium-3: Toward a Precise Measurement of the Neutron A 1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Parno, Diana Seymour

2011-04-01

The spin structure of protons and neutrons has been an open question for nearly twenty-five years, after surprising experimental results disproved the simple model in which valence quarks were responsible for nearly 100% of the nucleon spin. Diverse theoretical approaches have been brought to bear on the problem, but a shortage of precise data - especially on neutron spin structure - has prevented a thorough understanding. Experiment E06-014, conducted in Hall A of Jefferson Laboratory in 2009, presented an opportunity to add to the world data set for the neutron in the poorly covered valence-quark region. Jefferson Laboratory's highly polarizedmore » electron beam, combined with Hall A's facilities for a high-density, highly polarized 3He target, allowed a high-luminosity double-polarized experiment, while the large acceptance of the BigBite spectrometer gave coverage over a wide kinematic range: 0.15 < x < 0.95. In this work, we present the analysis of a portion of the E06-014 data, measured with an incident beam energy of 4.74 GeV and spanning 1.5 < Q 2 < 5.5 (GeV/c) 2. From these data, we extract the longitudinal asymmetry in virtual photon-nucleon scattering, A 1, on the 3He nucleus. Combined with the remaining E06-014 data, this will form the basis of a measurement of the neutron asymmetry A η 1 that will extend the kinematic range of the data available to test models of spin-dependent parton distributions in the nucleon.« less

Kinetics and dynamics of annealing during sub-gel phase formation in phospholipid bilayers

PubMed Central

Páli, Tibor; Bartucci, Rosa; Horváth, László I.; Marsh, Derek

1993-01-01

The saturation transfer electron spin resonance (STESR) spectra of spin-labeled phosphatidylcholine have been used to follow the kinetics of conversion from the gel phase to the sub-gel phase in aqueous bilayers of dipalmitoyl phosphatidylcholine. This is a simple, well-defined model system for lipid domain formation in membranes. The integrated intensity of the STESR spectrum from the chain-labeled lipid first increases and then decreases with time of incubation in the gel phase at 0°C. The first, more rapid phase of the kinetics is attributed to the conversion of germ nuclei to growth nuclei of the sub-gel phase. The increase in STESR intensity corresponds to the reduction in chain mobility of spin labels located in the gel phase at the boundaries of the growth nuclei and correlates with the increase in the diagnostic STESR line height ratios over this time range. The second, slower phase of the kinetics is attributed to growth of the domains of the sub-gel phase. The decrease in STESR intensity over this time regime corresponds to exclusion of the spin-labeled lipids from the tightly packed sub-gel phase and correlates quantitatively with calibrations of the spin label concentration dependence of the STESR intensity in the gel phase. The kinetics of formation of the sub-gel phase are consistent with the classical model for domain formation and growth. At 0°C, the half-time for conversion of germ nuclei to growth nuclei is ∼7.7 h and domain growth of the sub-gel phase is characterized by a rate constant of 0.025 h-1. The temperature dependence of the STESR spectra from samples annealed at 0°C suggests that the subtransition takes place via dissolution of sub-gel phase domains, possibly accompanied by domain fission. PMID:19431899

Uncertainties and understanding of experimental and theoretical results regarding reactions forming heavy and superheavy nuclei

NASA Astrophysics Data System (ADS)

Giardina, G.; Mandaglio, G.; Nasirov, A. K.; Anastasi, A.; Curciarello, F.; Fazio, G.

2018-02-01

Experimental and theoretical results of the PCN fusion probability of reactants in the entrance channel and the Wsur survival probability against fission at deexcitation of the compound nucleus formed in heavy-ion collisions are discussed. The theoretical results for a set of nuclear reactions leading to formation of compound nuclei (CNs) with the charge number Z = 102- 122 reveal a strong sensitivity of PCN to the characteristics of colliding nuclei in the entrance channel, dynamics of the reaction mechanism, and excitation energy of the system. We discuss the validity of assumptions and procedures for analysis of experimental data, and also the limits of validity of theoretical results obtained by the use of phenomenological models. The comparison of results obtained in many investigated reactions reveals serious limits of validity of the data analysis and calculation procedures.

Mastication induces long-term increases in blood perfusion of the trigeminal principal nucleus.

PubMed

Viggiano, A; Manara, R; Conforti, R; Paccone, A; Secondulfo, C; Lorusso, L; Sbordone, L; Di Salle, F; Monda, M; Tedeschi, G; Esposito, F

2015-12-17

Understanding mechanisms for vessel tone regulation within the trigeminal nuclei is of great interest because some headache syndromes are due to dysregulation of such mechanisms. Previous experiments on animal models suggest that mastication may alter neuron metabolism and blood supply in these nuclei. To investigate this hypothesis in humans, arterial spin-labeling magnetic resonance imaging (MRI) was used to measure blood perfusion within the principal trigeminal nucleus (Vp) and in the dorsolateral-midbrain (DM, including the mesencephalic trigeminal nucleus) in healthy volunteers, before and immediately after a mastication exercise consisting of chewing a gum on one side of the mouth for 1 h at 1 bite/s. The side preference for masticating was evaluated with a chewing test and the volume of the masseter muscle was measured on T1-weighted MRI scans. The results demonstrated that the mastication exercise caused a perfusion increase within the Vp, but not in the DM. This change was correlated to the preference score for the side where the exercise took place. Moreover, the basal Vp perfusion was correlated to the masseter volume. These results indicate that the local vascular tone of the trigeminal nuclei can be constitutively altered by the chewing practice and by strong or sustained chewing. Copyright © 2015 IBRO. Published by Elsevier Ltd. All rights reserved.

Measurement of key resonances for the 24Al(p ,γ )25Si reaction rate using in-beam γ -ray spectroscopy

NASA Astrophysics Data System (ADS)

Longfellow, B.; Gade, A.; Brown, B. A.; Richter, W. A.; Bazin, D.; Bender, P. C.; Bowry, M.; Elman, B.; Lunderberg, E.; Weisshaar, D.; Williams, S. J.

2018-05-01

Energy levels and branching ratios for the rp-process nucleus 25Si were determined from the reactions 9Be(26Si,25Si)X and 9Be(25Al,25Si)X using in-beam γ -ray spectroscopy with both high-efficiency and high-resolution detector arrays. Proton-unbound states at 3695(14) and 3802(11) keV were identified and assigned tentative spins and parities based on comparison to theory and the mirror nucleus. The 24Al(p ,γ )25Si reaction rate was calculated using the experimental states and states from charge-dependent USDA and USDB shell-model calculations with downward shifts of the 1 s1 /2 proton orbital to account for the observed Thomas-Ehrman shift, leading to a factor of 10-100 increase in rate for the temperature region of 0.22 GK as compared to a previous calculation. These shifts may be applicable to neighboring nuclei, impacting the proton capture rates in this region of the chart.

Comparison of magnetic resonance imaging sequences for depicting the subthalamic nucleus for deep brain stimulation.

PubMed

Nagahama, Hiroshi; Suzuki, Kengo; Shonai, Takaharu; Aratani, Kazuki; Sakurai, Yuuki; Nakamura, Manami; Sakata, Motomichi

2015-01-01

Electrodes are surgically implanted into the subthalamic nucleus (STN) of Parkinson's disease patients to provide deep brain stimulation. For ensuring correct positioning, the anatomic location of the STN must be determined preoperatively. Magnetic resonance imaging has been used for pinpointing the location of the STN. To identify the optimal imaging sequence for identifying the STN, we compared images produced with T2 star-weighted angiography (SWAN), gradient echo T2*-weighted imaging, and fast spin echo T2-weighted imaging in 6 healthy volunteers. Our comparison involved measurement of the contrast-to-noise ratio (CNR) for the STN and substantia nigra and a radiologist's interpretations of the images. Of the sequences examined, the CNR and qualitative scores were significantly higher on SWAN images than on other images (p < 0.01) for STN visualization. Kappa value (0.74) on SWAN images was the highest in three sequences for visualizing the STN. SWAN is the sequence best suited for identifying the STN at the present time.

Consequences of Relativistic Neutron Outflow beyond the Accretion Disks of Active Galaxies

NASA Astrophysics Data System (ADS)

Ekejiuba, I. E.; Okeke, P. N.

1993-05-01

Three channels of relativistic electron injection in the jets of extragalactic radio sources (EGRSs) are discussed. With the assumption that an active galactic nucleus (AGN) is powered by a spinning supermassive black hole of mass ~ 10(8) M_⊙ which sits at the center of the nucleus and ingests matter and energy through an accretion disk, a model for extracting relativistic neutrons from the AGN is forged. In this model, the inelastic proton--proton and proton--photon interactions within the accretion disk, of relativistic protons with background thermal protons and photons, respectively, produce copious amounts of relativistic neutrons. These neutrons travel ballistically for ~ 10(3gamma_n ) seconds and escape from the disk before they decay. The secondary particles produced from the neutron decays then interact with the ambient magnetic field and/or other particles to produce the radio emissions observed in the jets of EGRSs. IEE acknowledges the support of the World Bank and the Federal University of Technology, Yola, Nigeria as well as the hospitality of Georgia State University.

On the Dust Environment of Comet C/2012 S1 (ISON) from 12 AU Pre-perihelion to the End of its Activity around Perihelion

NASA Astrophysics Data System (ADS)

Moreno, F.; Pozuelos, F.; Aceituno, F.; Casanova, V.; Duffard, R.; López-Moreno, J. J.; Molina, A.; Ortiz, J. L.; Santos-Sanz, P.; Sota, A.; Diepvens, A.; Segundo, A. S.; Bell, C.; Labordena, C.; Bryssinck, E.; Cortés, E.; Reina, E.; García, F.; Gómez, F.; Limón, F.; Soldán, F.; Tifner, F.; Muler, G.; Almendros, I.; Aledo, J.; Bel, J.; Carrillo, J.; Castellano, J.; Curto, J.; Gaitan, J.; Salto, J. L.; Lopesino, J.; Lozano, J.; Hernández, J. F.; González, J. J.; Martín, J. L.; Aymamí, J. M.; Bosch, J. M.; Fernández, J. M.; Vidal, J. R.; Montoro, L.; Tremosa, L.; Campas, M.; Canales, O.; Dekelver, P. J.; Benavides, R.; Naves, R.; Castillo, R.; Climent, T.; Cupillari, T.; Yanamandra-Fisher, P.

2014-08-01

A Monte Carlo dust tail model has been applied to extract the dust environment parameters of the comet C/2012 S1 (ISON) from both Earth-based and SOHO LASCO C3 observations, performed from about six astronomical units (AU) inbound, to just after perihelion passage, when only a small portion of the original comet nucleus has survived in the form of a cloud of tiny particles. The early Afρ and image data are consistent with particle ejection from an extended active area located at latitudes 35°N to 90°N (for a prograde rotating nucleus), with the spin axis having a large obliquity (I ~ 70°). This configuration nicely fits the early images and Afρ data until 3.9 AU inbound, when the emission should become isotropic in order to fit the data. The analysis of LASCO images reveals that, assuming an original nucleus of RN = 500 m with ρ = 1000 kg m-3, at least half of its mass was vaporized when the comet was at about 17 R ⊙ inbound. We conclude that at that time the nucleus suffered a cataclysmic fragmentation releasing a huge amount of material of 2.3 ×1011 kg, equivalent to a sphere of 380 m in radius with density 1000 kg m-3. The surviving material after perihelion passage consists of very small dust particles of 0.1-50 μm in radius with a total mass of just 6.7×108 kg.

Signatures of triaxiality in low-spin spectra of 86Ge

NASA Astrophysics Data System (ADS)

Lettmann, M.; Werner, V.; Pietralla, N.; Doornenbal, P.; Obertelli, A.; Rodríguez, T. R.; Sieja, K.; Authelet, G.; Baba, H.; Calvet, D.; Château, F.; Chen, S.; Corsi, A.; Delbart, A.; Gheller, J.-M.; Giganon, A.; Gillibert, A.; Lapoux, V.; Motobayashi, T.; Niikura, M.; Paul, N.; Roussé, J.-Y.; Sakurai, H.; Santamaria, C.; Steppenbeck, D.; Taniuchi, R.; Uesaka, T.; Ando, T.; Arici, T.; Blazhev, A.; Browne, F.; Bruce, A.; Caroll, R. J.; Chung, L. X.; Cortés, M. L.; Dewald, M.; Ding, B.; Flavigny, F.; Franchoo, S.; Górska, M.; Gottardo, A.; Jungclaus, A.; Lee, J.; Linh, B. D.; Liu, J.; Liu, Z.; Lizarazo, C.; Momiyama, S.; Moschner, K.; Nagamine, S.; Nakatsuka, N.; Nita, C.; Nobs, C. R.; Olivier, L.; Patel, Z.; Podolyák, Zs.; Rudigier, M.; Saito, T.; Shand, C.; Söderström, P.-A.; Stefan, I.; Vaquero, V.; Wimmer, K.; Xu, Z.

2018-05-01

Low-spin states of neutron-rich 84,86,88Ge were measured by in-flight γ-ray spectroscopy at 270 MeV/u at the RIKEN-RIBF facility. The exotic beams have been produced by primary 238U in-flight fission reactions and impinged on the MINOS device. MINOS combines a 10-cm long LH2 target with a Time Projection Chamber (TPC) to reconstruct the reaction vertices. The reactions were selected by the BigRIPS and the ZeroDegree spectrometers for the incoming and outgoing channels, respectively. Emitted γ radiation was detected by the NaI-array DALI2. De-excitations from the {6}1+, {4}1,2+, and {2}1,2+ states of 84,86Ge and {4}1+ and {2}1,2+ states of 88Ge were observed. The data are compared to state-of-the-art shell model and beyond-mean-field calculations. Furthermore, a candidate for a {3}1+ state of 86Ge was identified. This state plays a key role in the discussion of ground-state triaxiality of 86Ge, along with other features of the low-energy level scheme. This work was published in [1].

a Truncated Spherical Shell Model for Nuclear Collective Excitations: Applications to the Odd Mass Systems, Neutron-Proton Systems and Other Topics.

NASA Astrophysics Data System (ADS)

Wu, Hua

One of the most elusive quantum system in nature is the nucleus, which is a strongly interacting many body system. In the hadronic (a la neutrons and protons) phase, the primary concern of this thesis, the nucleus' single particle excitations are intertwined with their various collective excitations. Although the underpinning of the nucleus is the spherical shell model, it is rendered powerless without a severe, but "intelligent" truncation of the infinite Hilbert space. The recently proposed Fermion Dynamical Symmetry Model (FDSM) is precisely such a truncation scheme and in which a symmetry-dictated turncation scheme is introduced in nuclear physics for the first time. In this thesis, extensions and explorations of the FDSM are made to specifically study the odd mass (where the most intricate mixing of the single particle and the collective excitations are observed) and the neutron-proton systems. In particular, we find that the previously successful phenomenological particle-rotor-model of the Copenhagen school can now be well understood microscopically via the FDSM. Furthermore, the well known Coriolis attenuation and variable moment of inertia effects are naturally understood from the model as well. A computer code FDU0 was written by one of us to study, for the first time, the numerical implications of the FDSM. Several collective modes were found even when the system does not admit a group chain description. In addition, the code is most suitable to study the connection between level statistical behavior (a al Gaussian Orthogonal Ensemble) and dynamical symmetry. It is found that there exist critical region of the interaction parameter space were the system behaves "chaotically". This information is certainly crucial to understanding quantum "chaotic" behavior. Also, some of the primitive assumptions of the FDSM are investigated and we concluded that the assumption of the quasi-spin behavior for the so-called abnormal parity particles is inadequate and needs to be extended. Suggestions of extensions are made. Finally, the newly developed physical quantity, the collective spin, is explored in terms of dynamical symmetries in the FDSM.

Results of the engineering run of the Coherent Neutrino Nucleus Interaction Experiment (CONNIE)

NASA Astrophysics Data System (ADS)

Aguilar-Arevalo, A.; Bertou, X.; Bonifazi, C.; Butner, M.; Cancelo, G.; Castañeda Vázquez, A.; Cervantes Vergara, B.; Chavez, C. R.; Da Motta, H.; D'Olivo, J. C.; Dos Anjos, J.; Estrada, J.; Fernandez Moroni, G.; Ford, R.; Foguel, A.; Hernández Torres, K. P.; Izraelevitch, F.; Kavner, A.; Kilminster, B.; Kuk, K.; Lima, H. P., Jr.; Makler, M.; Molina, J.; Moreno-Granados, G.; Moro, J. M.; Paolini, E. E.; Sofo Haro, M.; Tiffenberg, J.; Trillaud, F.; Wagner, S.

2016-07-01

The CONNIE detector prototype is operating at a distance of 30 m from the core of a 3.8 GWth nuclear reactor with the goal of establishing Charge-Coupled Devices (CCD) as a new technology for the detection of coherent elastic neutrino-nucleus scattering. We report on the results of the engineering run with an active mass of 4 g of silicon. The CCD array is described, and the performance observed during the first year is discussed. A compact passive shield was deployed around the detector, producing an order of magnitude reduction in the background rate. The remaining background observed during the run was stable, and dominated by internal contamination in the detector packaging materials. The in-situ calibration of the detector using X-ray lines from fluorescence demonstrates good stability of the readout system. The event rates with the reactor ON and OFF are compared, and no excess is observed coming from nuclear fission at the power plant. The upper limit for the neutrino event rate is set two orders of magnitude above the expectations for the standard model. The results demonstrate the cryogenic CCD-based detector can be remotely operated at the reactor site with stable noise below 2 e- RMS and stable background rates. The success of the engineering test provides a clear path for the upgraded 100 g detector to be deployed during 2016.

The functionally conserved nucleoporins Nup124p from fission yeast and the human Nup153 mediate nuclear import and activity of the Tf1 retrotransposon and HIV-1 Vpr.

PubMed

Varadarajan, Padmapriya; Mahalingam, Sundarasamy; Liu, Peiyun; Ng, Sarah Boon Hsi; Gandotra, Sheetal; Dorairajoo, Desmond Suresh Kumar; Balasundaram, David

2005-04-01

We report that the fission yeast nucleoporin Nup124p is required for the nuclear import of both, retrotransposon Tf1-Gag as well as the retroviral HIV-1 Vpr. Failure to import Tf1-Gag into the nucleus in a nup124 null mutant resulted in complete loss of Tf1 transposition. Similarly, nuclear import of HIV-1 Vpr was impaired in nup124 null mutant strains and cells became resistant to Vpr's cell-killing activity. On the basis of protein domain similarity, the human nucleoporin Nup153 was identified as a putative homolog of Nup124p. We demonstrate that in vitro-translated Nup124p and Nup153 coimmunoprecipitate Tf1-Gag or HIV-1 Vpr. Though full-length Nup153 was unable to complement the Tf1 transposition defect in a nup124 null mutant, we provide evidence that both nucleoporins share a unique N-terminal domain, Nup124p(AA264-454) and Nup153(AA448-634) that is absolutely essential for Tf1 transposition. Epigenetic overexpression of this domain in a wild-type (nup124(+)) background blocked Tf1 activity implying that sequences from Nup124p and the human Nup153 challenged the same pathway affecting Tf1 transposition. Our results establish a unique relationship between two analogous nucleoporins Nup124p and Nup153 wherein the function of a common domain in retrotransposition is conserved.

OPTESIM, a Versatile Toolbox for Numerical Simulation of Electron Spin Echo Envelope Modulation (ESEEM) that Features Hybrid Optimization and Statistical Assessment of Parameters

PubMed Central

Sun, Li; Hernandez-Guzman, Jessica; Warncke, Kurt

2009-01-01

Electron spin echo envelope modulation (ESEEM) is a technique of pulsed-electron paramagnetic resonance (EPR) spectroscopy. The analyis of ESEEM data to extract information about the nuclear and electronic structure of a disordered (powder) paramagnetic system requires accurate and efficient numerical simulations. A single coupled nucleus of known nuclear g value (gN) and spin I=1 can have up to eight adjustable parameters in the nuclear part of the spin Hamiltonian. We have developed OPTESIM, an ESEEM simulation toolbox, for automated numerical simulation of powder two- and three-pulse one-dimensional ESEEM for arbitrary number (N) and type (I, gN) of coupled nuclei, and arbitrary mutual orientations of the hyperfine tensor principal axis systems for N>1. OPTESIM is based in the Matlab environment, and includes the following features: (1) a fast algorithm for translation of the spin Hamiltonian into simulated ESEEM, (2) different optimization methods that can be hybridized to achieve an efficient coarse-to-fine grained search of the parameter space and convergence to a global minimum, (3) statistical analysis of the simulation parameters, which allows the identification of simultaneous confidence regions at specific confidence levels. OPTESIM also includes a geometry-preserving spherical averaging algorithm as default for N>1, and global optimization over multiple experimental conditions, such as the dephasing time ( ) for three-pulse ESEEM, and external magnetic field values. Application examples for simulation of 14N coupling (N=1, N=2) in biological and chemical model paramagnets are included. Automated, optimized simulations by using OPTESIM lead to a convergence on dramatically shorter time scales, relative to manual simulations. PMID:19553148

Rotationally induced surface slope-instabilities and the activation of CO2 activity on comet 103P/Hartley 2

NASA Astrophysics Data System (ADS)

Steckloff, Jordan K.; Graves, Kevin; Hirabayashi, Masatoshi; Melosh, H. Jay; Richardson, James E.

2016-07-01

Comet 103P/Hartley 2 has diurnally controlled, CO2-driven activity on the tip of the small lobe of its bilobate nucleus. Such activity is unique among the comet nuclei visited by spacecraft, and suggests that CO2 ice is very near the surface, which is inconsistent with our expectations of an object that thermophysically evolved for ∼45 million years prior to entering the Jupiter Family of comets. Here we explain this pattern of activity by showing that a very plausible recent episode of rapid rotation (rotation period of ∼11 [10-13] h) would have induced avalanches in Hartley 2's currently active regions that excavated down to CO2-rich ices and activated the small lobe of the nucleus. At Hartley 2's current rate of spindown about its principal axis, the nucleus would have been spinning fast enough to induce avalanches ∼3-4 orbits prior to the DIXI flyby (∼1984-1991). This coincides with Hartley 2's discovery in 1986, and implies that the initiation of CO2 activity facilitated the comet's discovery. During the avalanches, the sliding material would either be lofted off the surface by gas activity, or possibly gained enough momentum moving downhill (toward the tip of the small lobe) to slide off the tip of the small lobe. Much of this material would have failed to reach escape velocity, and would reimpact the nucleus, forming debris deposits. The similar size frequency distribution of the mounds observed on the surface of Hartley 2 and chunks of material in its inner coma suggest that the 20-40 m mounds observed by the DIXI mission on the surface of Hartley 2 are potentially these fallback debris deposits. As the nucleus spun down (rotation period increased) from a period of ∼11-18.34 h at the time of the DIXI flyby, the location of potential minima, where materials preferentially settle, migrated about the surface, allowing us to place relative ages on most of the terrains on the imaged portion of the nucleus.

Enhanced trigger for the NIFFTE fissionTPC in presence of high-rate alpha backgrounds

NASA Astrophysics Data System (ADS)

Bundgaard, Jeremy; Niffte Collaboration

2015-10-01

Nuclear physics and nuclear energy communities call for new, high precision measurements to improve existing fission models and design next generation reactors. The Neutron Induced Fission Fragment Tracking experiment (NIFFTE) has developed the fission Time Projection Chamber (fissionTPC) to measure neutron induced fission with unrivaled precision. The fissionTPC is annually deployed to the Weapons Neutron Research facility at Los Alamos Neutron Science Center where it operates with a neutron beam passing axially through the drift volume, irradiating heavy actinide targets to induce fission. The fissionTPC was developed at the Lawrence Livermore National Laboratory's TPC lab, where it measures spontaneous fission from radioactive sources to characterize detector response, improve performance, and evolve the design. To measure 244Cm, we've developed a fission trigger to reduce the data rate from alpha tracks while maintaining a high fission detection efficiency. In beam, alphas from 239Pu are a large background when detecting fission fragments; implementing the fission trigger will greatly reduce this background. The implementation of the cathode fission trigger in the fissionTPC will be presented along with a detailed study of its efficiency.

Shell Evolution towards 78Ni: Low-Lying States in 77Cu

NASA Astrophysics Data System (ADS)

Sahin, E.; Bello Garrote, F. L.; Tsunoda, Y.; Otsuka, T.; de Angelis, G.; Görgen, A.; Niikura, M.; Nishimura, S.; Xu, Z. Y.; Baba, H.; Browne, F.; Delattre, M.-C.; Doornenbal, P.; Franchoo, S.; Gey, G.; Hadyńska-KlÈ©k, K.; Isobe, T.; John, P. R.; Jung, H. S.; Kojouharov, I.; Kubo, T.; Kurz, N.; Li, Z.; Lorusso, G.; Matea, I.; Matsui, K.; Mengoni, D.; Morfouace, P.; Napoli, D. R.; Naqvi, F.; Nishibata, H.; Odahara, A.; Sakurai, H.; Schaffner, H.; Söderström, P.-A.; Sohler, D.; Stefan, I. G.; Sumikama, T.; Suzuki, D.; Taniuchi, R.; Taprogge, J.; Vajta, Z.; Watanabe, H.; Werner, V.; Wu, J.; Yagi, A.; Yalcinkaya, M.; Yoshinaga, K.

2017-06-01

The level structure of the neutron-rich 77Cu nucleus is investigated through β -delayed γ -ray spectroscopy at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. Ions of 77Ni are produced by in-flight fission, separated and identified in the BigRIPS fragment separator, and implanted in the WAS3ABi silicon detector array, surrounded by Ge cluster detectors of the EURICA array. A large number of excited states in 77Cu are identified for the first time by correlating γ rays with the β decay of 77Ni, and a level scheme is constructed by utilizing their coincidence relationships. The good agreement between large-scale Monte Carlo shell model calculations and experimental results allows for the evaluation of the single-particle structure near 78Ni and suggests a single-particle nature for both the 5 /21- and 3 /21- states in 77Cu, leading to doubly magic 78Ni.

Clustering and pasta phases in nuclear density functional theory

DOE PAGES

Schuetrumpf, Bastian; Zhang, Chunli; Nazarewicz, Witold

2017-05-23

Nuclear density functional theory is the tool of choice in describing properties of complex nuclei and intricate phases of bulk nucleonic matter. It is a microscopic approach based on an energy density functional representing the nuclear interaction. An attractive feature of nuclear DFT is that it can be applied to both finite nuclei and pasta phases appearing in the inner crust of neutron stars. While nuclear pasta clusters in a neutron star can be easily characterized through their density distributions, the level of clustering of nucleons in a nucleus can often be difficult to assess. To this end, we usemore » the concept of nucleon localization. We demonstrate that the localization measure provides us with fingerprints of clusters in light and heavy nuclei, including fissioning systems. Furthermore we investigate the rod-like pasta phase using twist-averaged boundary conditions, which enable calculations in finite volumes accessible by state of the art DFT solvers.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schuetrumpf, Bastian; Zhang, Chunli; Nazarewicz, Witold

Nuclear density functional theory is the tool of choice in describing properties of complex nuclei and intricate phases of bulk nucleonic matter. It is a microscopic approach based on an energy density functional representing the nuclear interaction. An attractive feature of nuclear DFT is that it can be applied to both finite nuclei and pasta phases appearing in the inner crust of neutron stars. While nuclear pasta clusters in a neutron star can be easily characterized through their density distributions, the level of clustering of nucleons in a nucleus can often be difficult to assess. To this end, we usemore » the concept of nucleon localization. We demonstrate that the localization measure provides us with fingerprints of clusters in light and heavy nuclei, including fissioning systems. Furthermore we investigate the rod-like pasta phase using twist-averaged boundary conditions, which enable calculations in finite volumes accessible by state of the art DFT solvers.« less

3D nanoscale imaging of the yeast, Schizosaccharomyces pombe, by full-field transmission X-ray microscopy at 5.4 keV.

PubMed

Chen, Jie; Yang, Yunhao; Zhang, Xiaobo; Andrews, Joy C; Pianetta, Piero; Guan, Yong; Liu, Gang; Xiong, Ying; Wu, Ziyu; Tian, Yangchao

2010-07-01

Three-dimensional (3D) nanoscale structures of the fission yeast, Schizosaccharomyces pombe, can be obtained by full-field transmission hard X-ray microscopy with 30 nm resolution using synchrotron radiation sources. Sample preparation is relatively simple and the samples are portable across various imaging environments, allowing for high-throughput sample screening. The yeast cells were fixed and double-stained with Reynold's lead citrate and uranyl acetate. We performed both absorption contrast and Zernike phase contrast imaging on these cells in order to test this method. The membranes, nucleus, and subcellular organelles of the cells were clearly visualized using absorption contrast mode. The X-ray images of the cells could be used to study the spatial distributions of the organelles in the cells. These results show unique structural information, demonstrating that hard X-ray microscopy is a complementary method for imaging and analyzing biological samples.

Temporal and Spatial Aspects of Gas Release During the 2010 Apparition of Comet 103P/Hartley-2

NASA Technical Reports Server (NTRS)

Mumma, M. J.; Bonev, B. P.; Villanueva, G. L.; Paganini, L.; DiSanti, M. A.; Gibb, E. L.; Keane, J. V.; Meech, K. J.; Blake, G. A.; Ellis, R. S.;

Results from the Super Cryogenic Dark Matter Search Experiment at Soudan

DOE PAGES

Agnese, R.; Aramaki, T.; Arnquist, I. J.; ...

2018-02-09

Here, we report the result of a blinded search for weakly interacting massive particles (WIMPs) using the majority of the SuperCDMS Soudan data set. With an exposure of 1690 kg d, a single candidate event is observed, consistent with expected backgrounds. This analysis (combined with previous Ge results) sets an upper limit on the spin-independent WIMP–nucleon cross section of 1.4×10 -44 (1.0×10 -44) cm 2 at 46 GeV/c 2. These results set the strongest limits for WIMP–germanium-nucleus interactions for masses >12 GeV/c 2.

Electromagnetic moments of 22F

NASA Astrophysics Data System (ADS)

Mihara, M.; Matsuta, K.; Komurasaki, J.; Hirano, H.; Nishimura, D.; Momota, S.; Ohtsubo, T.; Izumikawa, T.; Shimbara, Y.; Kubo, T.; Kameda, D.; Zhou, Dongmei; Zheng, Yongnan; Yuan, Daqing; Zhu, Shengyun; Kitagawa, A.; Kanazawa, M.; Torikoshi, M.; Sato, S.; Nagatomo, T.; Matsumiya, R.; Ishikawa, D.; Fukuda, M.; Minamisono, T.; Nojiri, Y.; Alonso, J. R.; Crebs, G. F.; Symons, T. J. M.

2010-03-01

The magnetic dipole (μ) and electric quadrupole (Q) moments of short-lived nucleus 22F (Iπ=4+, T=4.2s) have been measured for the first time by means of the β-NMR technique. A spin polarized 22F beam was produced through the charge exchange reaction of 22Ne and was implanted into single crysltals of NaF and MgF2 for μ and Q measurements, respectively. As a result, |μ(F22)|=(2.69443±0.00039)μ and |Q(F22)|=(3±2)mb was obtained. These values are well reproduced by the shell model calculations.

The effects of electrostatic charging on the dust distribution at Halley's Comet

NASA Technical Reports Server (NTRS)

Horanyi, M.; Mendis, D. A.

1986-01-01

The distribution of fine dust near Comet Halley at its 1910 and 1986 apparitions is investigated by means of computer simulations, taking the effects of EM forces due to the dust electrostatic charge into account. It is found that the nucleus spin period and orbital obliquity estimated by Sekanina and Larson (1984) from the 1910 observations are unaffected by these EM forces because the 1910 dust morphology involved mainly large grains. For 1986, the orientation of the smaller dust is shown to depend on the interplanetary magnetic field, with implications for the dust distribution encountered by the Halley probes.

Results from the Super Cryogenic Dark Matter Search Experiment at Soudan

NASA Astrophysics Data System (ADS)

Agnese, R.; Aramaki, T.; Arnquist, I. J.; Baker, W.; Balakishiyeva, D.; Banik, S.; Barker, D.; Basu Thakur, R.; Bauer, D. A.; Binder, T.; Bowles, M. A.; Brink, P. L.; Bunker, R.; Cabrera, B.; Caldwell, D. O.; Calkins, R.; Cartaro, C.; Cerdeño, D. G.; Chang, Y.; Chen, Y.; Cooley, J.; Cornell, B.; Cushman, P.; Daal, M.; Di Stefano, P. C. F.; Doughty, T.; Fascione, E.; Figueroa-Feliciano, E.; Fritts, M.; Gerbier, G.; Germond, R.; Ghaith, M.; Godfrey, G. L.; Golwala, S. R.; Hall, J.; Harris, H. R.; Hong, Z.; Hoppe, E. W.; Hsu, L.; Huber, M. E.; Iyer, V.; Jardin, D.; Jastram, A.; Jena, C.; Kelsey, M. H.; Kennedy, A.; Kubik, A.; Kurinsky, N. A.; Loer, B.; Lopez Asamar, E.; Lukens, P.; MacDonell, D.; Mahapatra, R.; Mandic, V.; Mast, N.; Miller, E. H.; Mirabolfathi, N.; Mohanty, B.; Morales Mendoza, J. D.; Nelson, J.; Orrell, J. L.; Oser, S. M.; Page, K.; Page, W. A.; Partridge, R.; Penalver Martinez, M.; Pepin, M.; Phipps, A.; Poudel, S.; Pyle, M.; Qiu, H.; Rau, W.; Redl, P.; Reisetter, A.; Reynolds, T.; Roberts, A.; Robinson, A. E.; Rogers, H. E.; Saab, T.; Sadoulet, B.; Sander, J.; Schneck, K.; Schnee, R. W.; Scorza, S.; Senapati, K.; Serfass, B.; Speller, D.; Stein, M.; Street, J.; Tanaka, H. A.; Toback, D.; Underwood, R.; Villano, A. N.; von Krosigk, B.; Welliver, B.; Wilson, J. S.; Wilson, M. J.; Wright, D. H.; Yellin, S.; Yen, J. J.; Young, B. A.; Zhang, X.; Zhao, X.; SuperCDMS Collaboration

2018-02-01

We report the result of a blinded search for weakly interacting massive particles (WIMPs) using the majority of the SuperCDMS Soudan data set. With an exposure of 1690 kg d, a single candidate event is observed, consistent with expected backgrounds. This analysis (combined with previous Ge results) sets an upper limit on the spin-independent WIMP-nucleon cross section of 1.4 ×10-44 (1.0 ×10-44) cm2 at 46 GeV /c2 . These results set the strongest limits for WIMP-germanium-nucleus interactions for masses >12 GeV /c2.

Results from the Super Cryogenic Dark Matter Search Experiment at Soudan

DOE Office of Scientific and Technical Information (OSTI.GOV)

Agnese, R.; Aramaki, T.; Arnquist, I. J.

Here, we report the result of a blinded search for weakly interacting massive particles (WIMPs) using the majority of the SuperCDMS Soudan data set. With an exposure of 1690 kg d, a single candidate event is observed, consistent with expected backgrounds. This analysis (combined with previous Ge results) sets an upper limit on the spin-independent WIMP–nucleon cross section of 1.4×10 -44 (1.0×10 -44) cm 2 at 46 GeV/c 2. These results set the strongest limits for WIMP–germanium-nucleus interactions for masses >12 GeV/c 2.

Collision of large dust particles with Suisei spacecraft

NASA Astrophysics Data System (ADS)

Uesugi, K.

1986-12-01

The spacecraft Suisei encountered Halley's comet at 13:05:49 UT on March 8, 1986. The closest approach distance to the comet was 151,000 km and during the time of closest approach, Suisei was hit twice by dust particles which were believed to come from the comet nucleus. Although Suisei has no dust counter or detector, the mass of these particles can be estimated by the analysis of attitude change of the spin-stabilized spacecraft perturbed by the collisions. The result shows that the minimum weight of the first particle should be several milligram and second one was several ten micrograms.

Results from the Super Cryogenic Dark Matter Search Experiment at Soudan

DOE Office of Scientific and Technical Information (OSTI.GOV)

Agnese, R.; Aramaki, T.; Arnquist, I. J.

We report the result of a blinded search for Weakly Interacting Massive Particles (WIMPs) using the full SuperCDMS Soudan dataset. With an exposure of 1690 kg days, a single event was observed after unblinding, consistent with expected backgrounds. This analysis (combined with previous Ge results) sets an upper limit on the spin-independent WIMP-nucleon cross section of 1.4x10^-44 (1.0x10^-44) cm^2 at 46 GeV/c^2 . These results set the strongest limits for WIMP-germanium-nucleus interactions for masses >12 GeV/c^2.

Structure of Sn 107 studied through single-neutron knockout reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cerizza, G.; Ayres, A.; Jones, K. L.

2016-02-04

The neutron-deficient nucleus Sn-107 has been studied by using the one-neutron knockout reaction. By measuring the decay gamma rays and momentum distributions of reaction residues, the spins of the ground, 5/2 +, and first-excited, 7/2 +, states of Sn-107 have been assigned by comparisons to eikonal-model reaction calculations. We also observed limits on the inclusive and exclusive cross sections and transitions due to neutron removals from below the N = 50 closed shell have been observed. New excited states up to 5.5 MeV in Sn-107 have been identified.