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Sample records for gamma spectrometry measurements

  1. Guide to plutonium isotopic measurements using gamma-ray spectrometry

    SciTech Connect

    Lemming, J.F.; Rakel, D.A.

    1982-08-26

    Purpose of this guide is to assist those responsible for plutonium isotopic measurements in the application of gamma-ray spectrometry. Objectives are to promote an understanding of the measurement process, including its limitations and applicability, by reviewing the general features of a plutonium spectrum and identifying the quantities which must be extracted from the data; to introduce state-of-the-art analysis techniques by reviewing four isotopic analysis packages and identifying their differences; to establish the basis for measurement control and assurance by discussing means of authenticating the performance of a measurement system; and to prepare for some specific problems encountered in plutonium isotopic analyses by providing solutions from the practical experiences of several laboratories. 29 references, 12 figures, 17 tables.

  2. Initial recommendations for restricting gamma-ray spectrometry measurements of radionuclides for on-site inspections

    SciTech Connect

    Buckley, W F; Kreek, S A; Wild, J F

    1998-11-06

    The US paper "Radionuclide Sampling, Sample Handling and Analytical Laboratory Equipment for Comprehensive Test Ban Treaty On-Site Inspections," CTBT/PC/V/OSI/WSII/PR/29 identified the radionuclides of interest to an OS1 as 144Ce, 147Nd, 141Ce, 149Ba140La), 95 Zr(95Nb), 131mXe, 133mXe, 133gXe, 135gXe, and 37Ar. All of these nuclides (except 37Ar) can be measured via some form of conventional or coincidence-based gamma-ray spectrometry. The non-gaseous radionuclides [144Ce, 147Nd, 141Ce, 140Ba(140La), and 95Zr(95Nb)] can be measured via conventional high-resolution gamma-ray spectrometry using a shielded, high-purity germanium (HPGe) detector. The gaseous radionuclides 131mXe, 133mXe, 133gXe, and 135gXe are best measured (after separation from their homologous elements) via a gamma & beta/electron coincidence technique such as that described in CTBT/WGB/TL-11/5 which could utilize either a HPGe or low-resolution (NaI(TI)) gamma-ray spectrometer to detect the gamma-ray/x-ray and a plastic scintillator to detect the beta particle/electron from the decay of the various Xe isotopes. The US paper CTBT/PC/V/IOSI/WSII/PR/29 (and other papers) identified a need to limit the information that can be extracted from high-resolution gamma-ray spectra to ensure that only information relevant to an OSI is accessible. The term "blinding" has been used to describe the need to limit the information available to the Inspection Team from the high-resolution gamma-ray measurement. A better term is "measurement restriction"; the need for restricting the information is particularly relevant to conventional high-resolution gamma-ray spectrometry measurements, but not to the gamma & beta/electron coincidence-type measurements

  3. Measurements of activation induced by environmental neutrons using ultra low-level gamma-ray spectrometry.

    PubMed

    Martínez Canet, M J; Hult, M; Köhler, M; Johnston, P N

    2000-03-01

    The flux of environmental neutrons is being studied by activation of metal discs of selected elements. Near the earth's surface the total neutron flux is in the order of 10(-2) cm(-2)s(-1), which gives induced activities of a few mBq in the discs. Initial results from this technique, involving activation at ground level for several materials (W, Au, Ta, In, Re, Sm, Dy and Mn) and ultra low-level gamma-ray spectrometry in an underground laboratory located at 500 m.w.e., are presented. Diffusion of environmental neutrons in water is also measured by activation of gold at different depths.

  4. Radioactivity measurements in the aquatic environment using in-situ and laboratory gamma-ray spectrometry.

    PubMed

    Eleftheriou, G; Tsabaris, C; Androulakaki, E G; Patiris, D L; Kokkoris, M; Kalfas, C A; Vlastou, R

    2013-12-01

    The in-situ underwater gamma-ray spectrometry method is validated by inter-comparison with laboratory method. Deployments of the spectrometer KATERINA on a submarine spring and laboratory measurements of water samples with HPGe detector were performed. Efficiency calibrations, Monte Carlo simulations and the Minimum Detectable Activity (MDA) estimations were realized. MDAs varied from 0.19 to 10.4 (lab) and 0.05 to 0.35 (in-situ) Bq/L, while activity concentrations differed from 7% (for radon progenies) up to 10% (for (40)K), between the two methods. PMID:24103707

  5. Measuring the radium quartet (228Ra, 226Ra, 224Ra, 223Ra) in seawater samples using gamma spectrometry.

    PubMed

    van Beek, P; Souhaut, M; Reyss, J-L

    2010-07-01

    Radium isotopes are widely used in marine studies (eg. to trace water masses, to quantify mixing processes or to study submarine groundwater discharge). While 228Ra and 226Ra are usually measured using gamma spectrometry, short-lived Ra isotopes (224Ra and 223Ra) are usually measured using a Radium Delayed Coincidence Counter (RaDeCC). Here we show that the four radium isotopes can be analyzed using gamma spectrometry. We report 226Ra, 228Ra, 224Ra, 223Ra activities measured using low-background gamma spectrometry in standard samples, in water samples collected in the vicinity of our laboratory (La Palme and Vaccarès lagoons, France) but also in seawater samples collected in the plume of the Amazon river, off French Guyana (AMANDES project). The 223Ra and 224Ra activities determined in these samples using gamma spectrometry were compared to the activities determined using RaDeCC. Activities determined using the two techniques are in good agreement. Uncertainties associated with the 224Ra activities are similar for the two techniques. RaDeCC is more sensitive for the detection of low 223Ra activities. Gamma spectrometry thus constitutes an alternate method for the determination of short-lived Ra isotopes.

  6. Measurement of uranium series radionuclides in rock and groundwater at the Koongarra ore deposit, Australia, by gamma spectrometry

    SciTech Connect

    Yanase, Nobuyuki; Sekine, Keiichi

    1995-12-31

    Gamma spectrometry without any self-absorption correction was developed to measure low energy gamma rays emitted by uranium and actinium series radionuclides in rock samples and groundwater residues collected at the Koongarra ore deposit, Australia. Thin samples were prepared to minimize the self-absorption by uranium in the samples. The present method gave standard deviations of 0.9 to 18% for the measurements of concentrations of uranium and actinium series radionuclides. The concentrations of {sup 238}U, {sup 230}Th and {sup 235}U measured by gamma spectrometry were compared with those by alpha spectrometry that requires a complicated chemical separation procedure. The results obtained by both methods were in fairly good agreement, and it was found that the gamma spectrometry is applicable to rock and groundwater samples having uranium content sup to 8.1% (10{sup 3} B1/g) and 3 Bq/l of {sup 238}U, respectively. The detection limits were calculated to be of the order of 10{sup {minus}2} Bq/g for rock samples and 10{sup {minus}1} Bq/l for groundwater samples. The concentrations of uranium and actinium series radionuclides can be determined precisely in these samples using gamma spectrometry without any self-absorption correction.

  7. A review of the nationwide proficiency test on natural radioactivity measurements by gamma spectrometry.

    PubMed

    Şahin, N K; Yeltepe, E; Yücel, Ü

    2016-03-01

    This study is the review of the first proficiency test on radioactivity measurement organized in Turkey by Sarayköy Nuclear Research and Training Center (SANAEM) of Turkish Atomic Energy Authority (TAEK) in 2013. The objective of the test was to determine (226)Ra, (232)Th and (40)K activity concentrations in natural soil samples using gamma-ray spectrometry. The bulk material consisting of uranium- and thorium-rich soil and sand was milled, mixed thoroughly and sieved. Homogeneity of the final mix was tested with 6 randomly taken samples. 16 proficiency test samples were distributed to 16 participating laboratories. 12 laboratories reported results. The results were evaluated on the accuracy and precision criteria adopted by the IAEA Proficiency Testing Group. The percentage of acceptable scores was 49%. Some recommendations have been provided to the laboratories to improve the quality of their results. It is planned to extend these proficiency tests periodically for various radionuclides in various matrices.

  8. A review of the nationwide proficiency test on natural radioactivity measurements by gamma spectrometry.

    PubMed

    Şahin, N K; Yeltepe, E; Yücel, Ü

    2016-03-01

    This study is the review of the first proficiency test on radioactivity measurement organized in Turkey by Sarayköy Nuclear Research and Training Center (SANAEM) of Turkish Atomic Energy Authority (TAEK) in 2013. The objective of the test was to determine (226)Ra, (232)Th and (40)K activity concentrations in natural soil samples using gamma-ray spectrometry. The bulk material consisting of uranium- and thorium-rich soil and sand was milled, mixed thoroughly and sieved. Homogeneity of the final mix was tested with 6 randomly taken samples. 16 proficiency test samples were distributed to 16 participating laboratories. 12 laboratories reported results. The results were evaluated on the accuracy and precision criteria adopted by the IAEA Proficiency Testing Group. The percentage of acceptable scores was 49%. Some recommendations have been provided to the laboratories to improve the quality of their results. It is planned to extend these proficiency tests periodically for various radionuclides in various matrices. PMID:26750585

  9. Airborne Gamma-Spectrometry in Switzerland

    SciTech Connect

    Butterweck, Gernot; Bucher, Benno; Rybach, Ladislaus

    2008-08-07

    Airborne gamma-spectrometry is able to obtain fast radiological information over large areas. The airborne gamma-spectrometry unit deployed in Switzerland by the Swiss National Emergency Operations Centre (NEOC) consists of a Swiss army Super Puma helicopter equipped with four NaI-Detectors with a total volume of 17 liters, associated electronics and a real-time data evaluation and mapping unit developed by the Swiss Federal Institute of Technology (ETH) and the Paul Scherrer Institut (PSI). The operational readiness of the airborne gamma-spectrometry system is validated in annual exercises of one week duration. Data from 2005 and 2006 exercises are represented in maps of {sup 137}Cs activity concentration for two towns located in southern and western Switzerland. An indicator of man-made radioactivity (MMGC ratio) is demonstrated for an area with four different types of nuclear installations. The intercomparison between airborne gamma-spectrometry and ground measurements showed good agreement between both methods.

  10. Monte Carlo simulation by GEANT 4 and GESPECOR of in situ gamma-ray spectrometry measurements.

    PubMed

    Chirosca, Alecsandru; Suvaila, Rares; Sima, Octavian

    2013-11-01

    The application of GEANT 4 and GESPECOR Monte Carlo simulation codes for efficiency calibration of in situ gamma-ray spectrometry was studied. The long computing time required by GEANT 4 prevents its use in routine simulations. Due to the application of variance reduction techniques, GESPECOR is much faster. In this code specific procedures for incorporating the depth profile of the activity were implemented. In addition procedures for evaluating the effect of non-homogeneity of the source were developed. The code was validated by comparison with test simulations carried out with GEANT 4 and by comparison with published results. PMID:23566809

  11. Measurement of gamma radiation levels in soil samples from Thanjavur using gamma-ray spectrometry and estimation of population exposure.

    PubMed

    Senthilkumar, B; Dhavamani, V; Ramkumar, S; Philominathan, P

    2010-01-01

    This study assesses the level of terrestrial gamma radiation and associated dose rates from the naturally occurring radionuclides (232)Th, (238)U and (40)K in 10 soil samples collected from Thanjavur (Tamil Nadu, India) using gamma-ray spectrometry. The activity profile of radionuclides has clearly showed the existence of low level activity in Thanjavur. The geometric mean activity concentrations of (232)Th, (238)U and (40)K is 42.9+/-9.4 Bq.kg(-1), 14.7+/-1.7 Bq.kg(-1) and 149.5+/-3.1 Bq.kg(-1) respectively are derived from all the soil samples studied. The activity concentration of (232)Th, (238)U and (40)K in soil is due to the presence of metamorphic rocks like shale, hornblende-biotite gneiss and quartzofeldspathic gneiss in these areas. Gamma absorbed dose rates in air outdoors were calculated to be in the range between 32 nGy.h(-1) and 59.1 nGy.h(-1) with an arithmetic mean of 43.3 +/-9 nGy.h(-1). This value is lesser than the population weighted world-averaged of 60 nGy.h(-1). Inhabitants of Thanjavur are subjected to external gamma radiation exposure (effective dose) ranging between 39.2 and 72.6 muSv.y(-1) with an arithmetic mean of 53.1+/-11 muSv.y(-1). The values of the external hazard index determined from the soil radioactivity of the study area are less than the recommended safe levels.

  12. Radioactivity of a Rock Profile from Rio do Rasto Formation Measured by High Resolution Gamma Spectrometry

    NASA Astrophysics Data System (ADS)

    Bastos, Rodrigo O.; Appoloni, Carlos R.; Pinese, José P. P.

    2011-08-01

    Natural occurring radionuclides are present in different concentrations in sedimentary rocks. Generally, their distribution correlates reasonably with their geo-physicochemical behavior during sediment deposition and rock consolidation. This fact permits to study some geological characteristics of the rocks by analyzing the radionuclide distribution in the rocks, as it might reflect the origin of the sediments, the depositional environment, and more recent events such as weathering and erosion. In this work, rocks from an exposed profile of the Rio do Rasto Formation were collected and analyzed in laboratory by high resolution gamma spectrometry for 226Ra, 232Th and 40K determination. It was employed a standard gamma ray spectrometry electronic chain, with a 66% relative efficiency HPGe detector. The efficiency calibration, as well as its validation, was accomplished with eight International Atomic Energy Agency certified samples. The outcrop exposes layers of sandstone and siltstone and, secondarily, claystone, with varying colors (gray, red and green). The rocks were collected along this profile, each of them was dried in the open air during 48 hours, grounded, sieved through 4 mm mesh and sealed in cylindrical recipients. The 226Ra, 232Th and 40K activity concentrations are presented, their distribution and the possible relations among activities are analyzed. The general pattern of radionuclides distribution respects well the hypotheses on geo-physicochemical behavior of radioactive elements.

  13. Improvements on Low Level Activity Gamma Measurements and X-ray Spectrometry at the CEA-MADERE Measurement Platform

    NASA Astrophysics Data System (ADS)

    Sergeyeva, Victoria; Domergue, Christophe; Destouches, Christophe; Girard, Jean Michel; Philibert, Hervé; Bonora, Jonathan; Thiollay, Nicolas; Lyoussi, Abdallah

    2016-02-01

    The CEA MADERE platform (Measurement Applied to DosimEtry in REactors) is a part of the Instrumentation Sensors and Dosimetry Laboratory (LDCI). This facility is dedicated to the specific activity measurements of solid and radioactive samples using Gamma and X-ray spectrometry. MADERE is a high-performance facility devoted to neutron dosimetry for experimental programs performed in CEA and for the irradiation surveillance programmes of PWR vessels. The MADERE platform is engaged in a continuous improvement process. Recently, two High Efficiency diodes have been integrated to the MADERE platform in order to manage the accurate low level activity measurements (few Bq per sample). This new equipment provides a good level of efficiency over the energy range from 60 keV to 2 MeV. The background continuum is reduced due to the use of a Ultra Low Background (ULB) lead shielding. Relative and absolute X-ray measurement techniques have been improved in order to facilitate absolute rhodium activity measurement (Rh103m) on solid samples. Additional efforts have been made to increase the accuracy of the relative niobium (Nb93m) activity measurement technique. The way of setting up an absolute measurement method for niobium is under investigation. After a presentation of the MADERE's measurement devices, this paper focuses on the technological options taken into account for the design of high efficiency measurement devices. Then, studies performed on X-ray measurement techniques are presented. Some details about the calculation of uncertainties and correction factors are also mentioned. Finally, future research and development axes are exposed.

  14. Assessment of measurement result uncertainty in determination of (210)Pb with the focus on matrix composition effect in gamma-ray spectrometry.

    PubMed

    Iurian, A R; Pitois, A; Kis-Benedek, G; Migliori, A; Padilla-Alvarez, R; Ceccatelli, A

    2016-03-01

    Reference materials were used to assess measurement result uncertainty in determination of (210)Pb by gamma-ray spectrometry, liquid scintillation counting, or indirectly by alpha-particle spectrometry, using its daughter (210)Po in radioactive equilibrium. Combined standard uncertainties of (210)Pb massic activities obtained by liquid scintillation counting are in the range 2-12%, depending on matrices and massic activity values. They are in the range 1-3% for the measurement of its daughter (210)Po using alpha-particle spectrometry. Three approaches (direct computation of counting efficiency and efficiency transfer approaches based on the computation and, respectively, experimental determination of the efficiency transfer factors) were applied for the evaluation of (210)Pb using gamma-ray spectrometry. Combined standard uncertainties of gamma-ray spectrometry results were found in the range 2-17%. The effect of matrix composition on self-attenuation was investigated and a detailed assessment of uncertainty components was performed. PMID:26653212

  15. The influence of exogenous conditions on mobile measured gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Dierke, C.; Werban, U.; Dietrich, P.

    2012-12-01

    In the past, gamma ray measurements have been used for geological surveys and exploration using airborne and borehole logging systems. For these applications, the relationships between the measured physical parameter - the concentration of natural gamma emitters 40K, 238U and 232Th - and geological origin or sedimentary developments are well described. Based on these applications and knowledge in combination with adjusted sensor systems, gamma ray measurements are used to derive soil parameters to create detailed soil maps e.g., in digital soil mapping (DSM) and monitoring of soils. Therefore, not only qualitative but also quantitative comparability is necessary. Grain size distribution, type of clay minerals and organic matter content are soil parameters which directly influence the gamma ray emitter concentration. Additionally, the measured concentration is influenced by endogenous processes like soil moisture variation due to raining events, foggy weather conditions, or erosion and deposition of material. A time series of gamma ray measurements was used to observe changes in gamma ray concentration on a floodplain area in Central Germany. The study area is characterised by high variations in grain size distribution and occurrence of flooding events. For the survey, we used a 4l NaI(Tl) detector with GPS connection mounted on a sledge, which is towed across the field sites by a four-wheel-vehicle. The comparison of data from different time steps shows similar structures with minor variation between the data ranges and shape of structures. However, the data measured during different soil moisture contents differ in absolute value. An average increase of soil moisture of 36% leads to a decrease of Th (by 20%), K (by 29%), and U (by 41%). These differences can be explained by higher attenuation of radiation during higher soil moisture content. The different changes in nuclide concentration will also lead to varying ratios. We will present our experiences concerning

  16. Optimization of measure parameters for an X- and gamma-ray spectrometry portable system

    NASA Astrophysics Data System (ADS)

    Fernandes, Jaquiel S.; Appoloni, Carlos R.

    2008-01-01

    In order to optimize the use of a system for in situ gamma ( γ)- and X-ray spectrometry composed of a 3×3×1 mm 3 Cadmium Telluride (CdTe) detector with respect to the detection of low-activity radioactive sources, a two level factorial planning was accomplished, involving three factors that could modify the system response. This planning was made with a 137Cs punctual source, analyzing the X-ray energy line of 32 keV from 137mBa. It was concluded that, for the system optimization, the best configuration for the involved parameters was to work with the detector at temperature of -22 °C, shaping time of 3 μs and rise time discrimination (RTD) with value 3.

  17. The use of difference spectra with a filtered rolling average background in mobile gamma spectrometry measurements

    NASA Astrophysics Data System (ADS)

    Cresswell, A. J.; Sanderson, D. C. W.

    2009-08-01

    The use of difference spectra, with a filtering of a rolling average background, as a variation of the more common rainbow plots to aid in the visual identification of radiation anomalies in mobile gamma spectrometry systems is presented. This method requires minimal assumptions about the radiation environment, and is not computationally intensive. Some case studies are presented to illustrate the method. It is shown that difference spectra produced in this manner can improve signal to background, estimate shielding or mass depth using scattered spectral components, and locate point sources. This approach could be a useful addition to the methods available for locating point sources and mapping dispersed activity in real time. Further possible developments of the procedure utilising more intelligent filters and spatial averaging of the background are identified.

  18. Measurement of the Modified Conversion Ratio of 238U by Gamma-Ray Spectrometry on AN Irradiated Fuel Pin

    NASA Astrophysics Data System (ADS)

    Hudelot, J. P.; Fougeras, P.; Cathalau, S.

    2003-06-01

    Within the frameworks of plutonium recycling, of transmutation, of waste management and of the increase of fuel loading length, controlling and improving the accuracy on 238U conversion ratio becomes necessary. Indeed, 238U neutron capture generates transuranian elements as for instance the isotopes of plutonium, americium or curium. This study focuses on a new technique for measuring by gamma-spectrometry, the modified conversion ratio of 238U defined as the ratio of the capture rate of 238U to the total fission rate, in an irradiated fuel pin of a critical assembly.

  19. Continuous measurement of radiation from radionuclides deposited on the ground using in situ gamma-ray spectrometry.

    PubMed

    Mirsch, M; Barth, J; Dalheimer, A; Steinkopff, T

    2014-08-01

    Until recently, in situ measurements in a network of radiation-measuring sites at the Deutscher Wetterdienst could only be started if all components had been put up in an instrumentation shelter and the detector had been cooled for ∼6 h. Within a project on partial automation of radioactivity monitoring, it has now become possible to permanently equip the measuring sites, i.e. the instrumentation shelter, with the components for in situ gamma-ray spectrometry. The cooling technology of the detectors changed from liquid nitrogen based to an electric system and the instrumentation shelters could be fixed with air conditioning to minimise the influence of changes in the outside temperature. PMID:24812073

  20. The radioactivity measurements in soils and fertilizers using gamma spectrometry technique.

    PubMed

    Boukhenfouf, Wassila; Boucenna, Ahmed

    2011-04-01

    Because of their mineral content, soils are naturally radioactive and one of the sources of radioactivity other than those of natural origin is mainly due to the extensive use of fertilizers. The main aim of this paper is to evaluate the fluxes of natural radionuclides in local production of phosphate fertilizers to determine the content of radioactivity in several commercial fertilizers produced in Algeria and to estimate their radiological impact in a cultivated soil even for the long-term exposure due to their application. For these purposes, virgin and fertilized soils were collected from outlying Setif region in Algeria and from phosphate fertilizers used in this area. Gamma spectrometry was exploited to determine activity concentration due to naturally occurring (226)Ra, (232)Th and (40)K in five types of samples (two different sorts of fertilizers, virgin and fertilized soils and well water used for irrigation) taken from Setif's areas. The results show that these radionuclides were present in an average concentration of 134.7 ± 24.1, 131.8 ± 16.7, 11644 ± 550 Bq/kg for the first fertilizer NPK and 190.3 ± 30, 117.2 ± 10.3, 5312 ± 249 Bq/kg for the second fertilizer (NPKs). For the virgin and the fertilized soils, the corresponding values were respectively 47.01 ± 7.3, 33 ± 7, 329.4 ± 19.7 Bq/kg and 53.2 ± 10.6, 50.0 ± 7, 311.4 ± 18.7 Bq/kg. For well water, the values were 1.93 and 0.12 Bq/kg; however the third value was below the Minimum Detectable Activity (MDA). The radium equivalent activity (Raeq) and the representative level index I(γr) for all samples were also calculated. The data were discussed and compared with those given in the literature.

  1. Simultaneous measurements of indoor radon, radon-thoron progeny and high-resolution gamma spectrometry in Greek dwellings.

    PubMed

    Clouvas, A; Xanthos, S; Antonopoulos-Domis, M

    2006-01-01

    Simultaneous indoor radon, radon-thoron progeny and high-resolution in situ gamma spectrometry measurements, with portable high-purity Ge detector were performed in 26 dwellings of Thessaloniki, the second largest town of Greece, during March 2003-January 2005. The radon gas was measured with an AlphaGUARD ionisation chamber (in each of the 26 dwellings) every 10 min, for a time period between 7 and 10 d. Most of the values of radon gas concentration are between 20 and 30 Bq m(-3), with an arithmetic mean of 34 Bq m(-3). The maximum measured value of radon gas concentration is 516 Bq m(-3). The comparison between the radon gas measurements, performed with AlphaGUARD and short-term electret ionisation chamber, shows very good agreement, taking into account the relative short time period of the measurement and the relative low radon gas concentration. Radon and thoron progeny were measured with a SILENA (model 4s) instrument. From the radon and radon progeny measurements, the equilibrium factor F could be deduced. Most of the measurements of the equilibrium factor are within the range 0.4-0.5. The mean value of the equilibrium factor F is 0.49 +/- 0.10, i.e. close to the typical value of 0.4 adopted by UNSCEAR. The mean equilibrium equivalent thoron concentration measured in the 26 dwellings is EEC(thoron) = 1.38 +/- 0.79 Bq m(-3). The mean equilibrium equivalent thoron to radon ratio concentration, measured in the 26 dwellings, is 0.1 +/- 0.06. The mean total absorbed dose rate in air, owing to gamma radiation, is 58 +/- 12 nGy h(-1). The contribution of the different radionuclides to the total indoor gamma dose rate in air is 38% due to 40K, 36% due to thorium series and 26% due to uranium series. The annual effective dose, due to the different source terms (radon, thoron and external gamma radiation), is 1.05, 0.39 and 0.28 mSv, respectively. PMID:16410290

  2. Spatially-Dependent Measurements of Surface and Near-Surface Radioactive Material Using In situ Gamma Ray Spectrometry (ISGRS) For Final Status Surveys

    SciTech Connect

    J. A. Chapman, A. J. Boerner, E. W. Abelquist

    2006-11-15

    In-situ, high-resolution gamma-ray spectrometry (ISGRS) measurements were conducted at the Oak Ridge Institute for Science and Education (ORISE) field laboratory in Oak Ridge, Tennessee. The purpose of these tests was to provide analytical data for assessing how “fit for use” this technology is for detecting discrete particles in soil.

  3. In situ gamma spectrometry measurements and Monte Carlo computations for the detection of radioactive sources in scrap metal.

    PubMed

    Clouvas, A; Xanthos, S; Takoudis, G; Potiriadis, C; Silva, J

    2005-02-01

    A very limited number of field experiments have been performed to assess the relative radiation detection sensitivities of commercially available equipment used to detect radioactive sources in recycled metal scrap. Such experiments require the cooperation and commitment of considerable resources on the part of vendors of the radiation detection systems and the cooperation of a steel mill or scrap processing facility. The results will unavoidably be specific to the equipment tested at the time, the characteristics of the scrap metal involved in the tests, and to the specific configurations of the scrap containers. Given these limitations, the use of computer simulation for this purpose would be a desirable alternative. With this in mind, this study sought to determine whether Monte Carlo simulation of photon flux energy distributions resulting from a radiation source in metal scrap would be realistic. In the present work, experimental and simulated photon flux energy distributions in the outer part of a truck due to the presence of embedded radioactive sources in the scrap metal load are compared. The experimental photon fluxes are deduced by in situ gamma spectrometry measurements with portable Ge detector and the calculated ones by Monte Carlo simulations with the MCNP code. The good agreement between simulated and measured photon flux energy distributions indicate that the results obtained by the Monte Carlo simulations are realistic.

  4. Applicability study of using in-situ gamma-ray spectrometry technique for 137Cs and 210Pb(ex) inventories measurement in grassland environments.

    PubMed

    Li, Junjie; Li, Yong; Wang, Yanglin; Wu, Jiansheng; Funk, Roger; Hoffmann, Carsten

    2010-06-01

    In-situ measurement of fallout radionuclides (137)Cs and (210)Pb(ex) has the potential to assess soil erosion and sedimentation rapidly. In this study, inventories of (137)Cs and (210)Pb(ex) in the soil of Inner Mongolia grassland were measured using an In-situ Object Counting System (ISOCS). The results from the field study indicate that in-situ gamma-ray spectrometry has the following advantages over traditional laboratory measurements: no extra time is required for sample collection, no reference inventories are required, more economic, prompt availability of the results, the ability to average radionuclide inventory over a large area, and high precision. PMID:20133146

  5. Methods for spectral interference corrections for direct measurements of 234U and 230Th in materials by gamma-ray spectrometry.

    PubMed

    Yücel, H; Solmaz, A N; Köse, E; Bor, D

    2010-03-01

    When the high-resolution gamma-ray spectrometry was used in the analysis of (234)U and (230)Th in samples, there is a much more need to correct for the measured activity results of (234)U and (230)Th mainly due to self-absorption effects and the interfering lines from (226)Ra, (235)U, (238)U and their decay products that often might be present in the samples. Therefore, in the present study, the methods for the spectral interference corrections for the analytical peaks of (234)U and (230)Th are suggested to take into account the contributions of the overlapping gamma rays to these peaks. For the method validation, direct gamma-ray spectrometric measurements were carried out using certified reference materials (CRM) by use of a 76.5 % n-type Ge detector. The activities measured for the CRM samples were corrected for spectral interferences, self-absorption and true coincidence-summing (TCS) effects. The obtained results indicate that ignoring of the contribution of the interference gamma rays to the main analytical peak at 53.2 keV of (234)U leads to a lager systematic error of 87.3-90.4 % for the measured activities of (234)U, and similarly if one ignores the contributions of the interference gamma rays to the main analytical peak at 67.7 keV of (230)Th, this leads to a much smaller systematic error of 2.1-2.7 % for the activities of (230)Th. Therefore, the required correction factors for spectral interferences to the analytical peaks of (234)U and (230)Th are not negligible and thus they should also be considered besides necessary self-absorption factors to determine more accurate activities in the samples. On the other hand, it is estimated that although the TCS effects on the main analytical peaks of both (234)U and (230)Th are negligibly small, those TCS correction factors for their interference gamma rays to these peaks should be taken into account when direct measurements are performed in a close-counting geometry condition. Otherwise, the resulted activities

  6. Measurement of gamma radiation levels in soil samples from Thanjavur using γ-ray spectrometry and estimation of population exposure

    PubMed Central

    Senthilkumar, B.; Dhavamani, V.; Ramkumar, S.; Philominathan, P.

    2010-01-01

    This study assesses the level of terrestrial gamma radiation and associated dose rates from the naturally occurring radionuclides 232Th, 238U and 40K in 10 soil samples collected from Thanjavur (Tamil Nadu, India) using γ-ray spectrometry. The activity profile of radionuclides has clearly showed the existence of low level activity in Thanjavur. The geometric mean activity concentrations of 232Th, 238U and 40K is 42.9±9.4 Bq.kg−1, 14.7±1.7 Bq.kg−1 and 149.5±3.1 Bq.kg−1 respectively are derived from all the soil samples studied. The activity concentration of 232Th, 238U and 40K in soil is due to the presence of metamorphic rocks like shale, hornblende-biotite gneiss and quartzofeldspathic gneiss in these areas. Gamma absorbed dose rates in air outdoors were calculated to be in the range between 32 nGy.h−1 and 59.1 nGy.h−1 with an arithmetic mean of 43.3 ±9 nGy.h−1. This value is lesser than the population weighted world-averaged of 60 nGy.h−1. Inhabitants of Thanjavur are subjected to external gamma radiation exposure (effective dose) ranging between 39.2 and 72.6 μSv.y−1 with an arithmetic mean of 53.1±11 μSv.y−1. The values of the external hazard index determined from the soil radioactivity of the study area are less than the recommended safe levels. PMID:20177570

  7. Spectral interference corrections for the measurement of (238)U in materials rich in thorium by a high resolution gamma-ray spectrometry.

    PubMed

    Yücel, H; Solmaz, A N; Köse, E; Bor, D

    2009-11-01

    In this study, the spectral interferences are investigated for the analytical peaks at 63.3 keV of (234)Th and 1001.0 keV of (234m)Pa, which are often used in the measurement of (238)U activity by the gamma-ray spectrometry. The correction methods are suggested to estimate the net peak areas of the gamma-rays overlapping the analytical peaks, due to the contribution of (232)Th that may not be negligible in materials rich in natural thorium. The activity results for the certified reference materials (CRMs) containing U and Th were measured with a well type Ge detector. The self-absorption and true coincidence-summing (TCS) effects were also taken into account in the measurements. It is found that ignoring the contributions of the interference gamma-rays of (232)Th and (235)U to the mixed peak at 63.3 keV of (234)Th ((238)U) leads to the remarkably large systematic influence of 0.8-122% in the measured (238)U activity, but in case of ignoring the contribution of (232)Th via the interference gamma-ray at 1000.7 keV of (228)Ac to the mixed peak at 1001 keV of (234m)Pa ((238)U) results in relatively smaller systematic influence of 0.05-3%, depending on thorium contents in the samples. The present results showed that the necessary correction for the spectral interferences besides self-absorption and TCS effects is also very important to obtain more accurate (238)U activity results. Additionally, if one ignores the contribution of (232)Th to both (238)U and (40)K activities in materials, the maximum systematic influence on the effective radiation dose is estimated to be ~6% and ~1% via the analytical peaks at 63.3 and 1001 keV for measurement of the (238)U activity, respectively. PMID:19683454

  8. Photon energy conversion efficiency in gamma-ray spectrometry.

    PubMed

    Švec, Anton

    2016-01-01

    Photon energy conversion efficiency coefficient is presented as the ratio of total energy registered in the collected spectrum to the emitted photon energy. This parameter is calculated from the conventional gamma-ray histogram and in principle is not affected by coincidence phenomena. This feature makes it particularly useful for calibration and measurement of radionuclide samples at close geometries. It complements the number of efficiency parameters used in gamma-ray spectrometry and can partly change the view as to how the gamma-ray spectra are displayed and processed.

  9. A method for determining the analytical form of a radionuclide depth distribution using multiple gamma spectrometry measurements.

    PubMed

    Dewey, Steven Clifford; Whetstone, Zachary David; Kearfott, Kimberlee Jane

    2011-06-01

    When characterizing environmental radioactivity, whether in the soil or within concrete building structures undergoing remediation or decommissioning, it is highly desirable to know the radionuclide depth distribution. This is typically modeled using continuous analytical expressions, whose forms are believed to best represent the true source distributions. In situ gamma ray spectroscopic measurements are combined with these models to fully describe the source. Currently, the choice of analytical expressions is based upon prior experimental core sampling results at similar locations, any known site history, or radionuclide transport models. This paper presents a method, employing multiple in situ measurements at a single site, for determining the analytical form that best represents the true depth distribution present. The measurements can be made using a variety of geometries, each of which has a different sensitivity variation with source spatial distribution. Using non-linear least squares numerical optimization methods, the results can be fit to a collection of analytical models and the parameters of each model determined. The analytical expression that results in the fit with the lowest residual is selected as the most accurate representation. A cursory examination is made of the effects of measurement errors on the method. PMID:21482447

  10. Measurement of natural radioactivity in building materials of Namakkal, Tamil Nadu, India using gamma-ray spectrometry.

    PubMed

    Ravisankar, R; Vanasundari, K; Chandrasekaran, A; Rajalakshmi, A; Suganya, M; Vijayagopal, P; Meenakshisundaram, V

    2012-04-01

    The natural level of radioactivity in building materials is one of the major causes of external exposure to γ-rays. The primordial radionuclides in building materials are one of the sources of radiation hazard in dwellings made of these materials. By the determination of the radioactivity level in building materials, the indoor radiological hazard to human health can be assessed. This is an important precautionary measure whenever the dose rate is found to be above the recommended limits. The aim of this work was to measure the specific activity concentration of (226)Ra, (232)Th and (40)K in commonly used building materials from Namakkal, Tamil Nadu, India, using gamma-ray spectrometer. The radiation hazard due to the total natural radioactivity in the studied building materials was estimated by different approaches. The concentrations of the natural radionuclides and the radium equivalent activity in studied samples were compared with the corresponding results of different countries. From the analysis, it is found that these materials may be safely used as construction materials and do not pose significant radiation hazards.

  11. Concentrations and their ratio of (222)Rn decay products in rainwater measured by gamma-ray spectrometry using a low-background Ge detector.

    PubMed

    Takeyasu, Masanori; Iida, Takao; Tsujimoto, Tadashi; Yamasaki, Keizo; Ogawa, Yoshihiro

    2006-01-01

    The concentrations and the concentration ratios of individual short-lived (222)Rn decay products ((214)Pb and (214)Bi) in rainwater were measured at Kumatori village (34.39 degrees N, 135.35 degrees E, approximately 70 m above sea level) in Osaka, Japan, by gamma-ray spectrometry using a low-background Ge detector. The dependence of the time variations of the concentrations and their ratios on rainfall rate was investigated. It was observed that the concentrations were negatively correlated with the rainfall rate in some rainfall events, and that there was no clear correlation in other rainfall events. The changes in the dependence of the concentration on the rainfall rate occurred after the passage of a cold front during a single rainfall event. The concentration ratios showed a weak negative correlation with the rainfall rate for most of the observed rainfall events. A scavenging model was designed in this study in order to explain the observation results. Based on the relationship between the concentrations of (214)Pb and (214)Bi in the rainwater and the rainfall rate for an individual rainfall event, the increase in the environmental gamma-ray dose rate from (214)Pb and (214)Bi deposited on the ground was calculated, and the calculated increase agreed well with that observed by the in situ measurement on flat ground. PMID:16530896

  12. The natural radioactivity measurements in coastal sediment samples along the East Coast of Tamilnadu using gamma spectrometry technique

    SciTech Connect

    Chandramohan, J.; Tholkappian, M.; Harikrishnan, N.; Ravisankar, R.

    2015-08-28

    The natural radioactivity concentration in beach sediment samples collected from Pattipulam to Devanampattinam of East Coast of Tamilnadu have been determined by NaI (TI) gamma ray spectrometer. The specific activity concentrations range from ≤ 2.21 (BDL) to 37.02 Bq kg{sup −1} with a mean of 3.79 Bqkg{sup −1} for {sup 238}U, ≤ 2.11 (BDL) to 643.77 Bqkg{sup −1} with a mean of 49.60 Bqkg{sup −1} for {sup 232}Th and 300.34 Bqkg{sup −1} to 449.08 Bqkg{sup −1} with a mean of 360.23 Bqkg{sup −1} for {sup 40}K. The potential radiological hazards due to natural radionuclides content such as Radium Equivalent activity (Ra{sub eq}), Representative level index (RLI), External hazard index (H{sub ex}), absorbed gamma does rate (D{sub R}), and Annual effective dose rate (AEDR) are estimated to assess the radiation hazard associated with the sediments. The obtained data are compared with the recommended safety limits and international approved values. All the values are well below the recommended safety limits indicating that radiation levels do not poses any significant health hazard to the public in the area as a result of the natural radioactivity of beach sediments. This study may help the baseline data for more extensive works in the same subjects of future studies.

  13. Composite mapping experiences in airborne gamma spectrometry.

    PubMed

    Bucher, B

    2014-08-01

    During an international intercomparison exercise of airborne gamma spectrometry held in Switzerland 2007 teams from Germany, France and Switzerland were proving their capabilities. One of the tasks was the composite mapping of an area around Basel. Each team was mainly covering the part of its own country at its own flying procedures. They delivered the evaluated data in a data format agreed in advance. The quantities to be delivered were also defined in advance. Nevertheless, during the process to put the data together a few questions raised: Which dose rate was meant? Had the dose rate to be delivered with or without cosmic contribution? Activity per dry or wet mass? Which coordinate system was used? Finally, the data could be put together in one map. For working procedures in case of an emergency, quantities of interest and exchange data format have to be defined in advance. But the procedures have also to be proved regularly. PMID:24664949

  14. Measurement of activity concentrations of natural radionuclides in the topsoil of IITA Ibadan by gamma-ray spectrometry.

    PubMed

    Okeyode, I C; Farai, I P

    2007-09-01

    The activity concentrations of the natural radionuclides in the soils at the International Institute of Tropical Agriculture, (IITA), Idi-Ose, Moniya, Ibadan, Nigeria were investigated using a NaI (Tl) scintillation detector coupled with a Canberra series 10 plus multichannel analyser as the detecting device for gamma scintillation spectroscopy. The whole area was divided into grids and soil samples were collected from the points of intersection of the grids. The average activity concentrations obtained for the three radionuclides (40K, 238U and 232Th) were 180.08 +/- 90.54 Bq kg(-1) for 40K, 8.901 +/- 5.063 Bq kg(-1) for 238U and 11.01 +/- 7.686 Bq kg(-1) for 232Th. The average values of the absorbed dose rate for each radionuclide were found to be 7.33 nGy h(-1) for 232Th, 7.55 nGy h(-1) for 40K and 3.82 nGy h(-1) for 238U. The average (baseline) of the total absorbed dose rate was found to be 18.72 +/- 8.11 nGy h(-1). The baseline average outdoor annual effective dose equivalent at IITA due to the concentrations of the radionuclides was found to be 22.95 +/- 9.94 microSv y(-1). This value is low compared to the world average of 70 microSv y(-1) specified by UNSCEAR for an outdoor effective dose. Hence the probability of occurrence of any of the health effects of radiation is low.

  15. In situ gamma-spectrometry intercomparison exercise in Salzburg, Austria

    NASA Astrophysics Data System (ADS)

    Lettner, H.; Andrasi, A.; Hubmer, A. K.; Lovranich, E.; Steger, F.; Zombori, P.

    1996-02-01

    In situ gamma-spectrometry has become a useful method of assessing the nuclide concentrations of man-made and natural gamma-emitters in the soil. For the quality assurance of the measurements, periodically conducted intercomparison exercises are essential. Therefore exercises were organized in different European countries since 1990, the last one was conducted in Salzburg, Austria in September 1994. The participation of 27 measurement teams from all over Europe emphasizes the importance of the intercomparison. Salzburg was selected because the Province of Salzburg, Austria was among the most heavily contaminated regions outside the former USSR by the Chernobyl fallout. Two different typical sites were selected for the measurements: Site 1 was inside the urban area of Salzburg on intensively used grassland which had not been tilled since the deposition of the fallout. This site is representative for intensively used agricultural regions in the Province of Salzburg. Site 2 was in the mountainous regions of the Hohe Tauern at an elevated altitude of 1600 m, representing the agricultural soil- and contamination conditions of the Alpine regions in the Tauern. The two sites differ significantly in terms of soil characteristics, a crucial parameter for the evaluation of in situ gamma-spectra. The participants used different approaches for the evaluation of the gamma-spectra in terms of considering the depth distribution. In the paper the results from the 24 European teams are presented.

  16. In-situ gamma spectrometry in environmental monitoring.

    PubMed

    Kluson, J

    2010-01-01

    In-situ gamma spectrometry (scintillation or semiconductor) can be used effectively for monitoring natural and man-made radionuclide concentrations, together with the corresponding photon fields, in the environment and in workplaces. It is applied in operational and emergency monitoring of nuclear facilities, waste storage facilities and the uranium industry, in radioactive contamination measurements and mapping, environmental, radiohygienic and radiation safety studies, etc. Methods for processing and interpreting data, experimental techniques (ground or airborne arrangement), calibration and verification and examples of applications are discussed in this paper. PMID:20022255

  17. Gamma-ray spectrometry of LDEF samples

    SciTech Connect

    Winn, W.G.

    1991-01-01

    A total of 31 samples from the Long Duration Exposure Facility (LDEF), including materials of aluminum, vanadium, and steel trunnions were analyzed by ultra-low-level gamma spectroscopy. The study quantified particle induced activations of (sup 22)Na, {sup 46}Sc, {sup 51}Cr, {sup 54}Mn, {sup 56}Co, {sup 57}Co, {sup 58}Co, and {sup 60}Co. The samples of trunnion sections exhibited increasing activity toward the outer end of the trunnion and decreasing activity toward its radial center. The trunnion sections did not include end pieces, which have been reported to collect noticeable {sup 7}Be on their leading surfaces. No significant {sup 7}Be was detected in the samples analyzed. The Underground Counting Facility at Savannah River Laboratory (SRL) was used in this work. The facility is 50 ft. underground, constructed with low-background shielding materials, and operated as a clean room. The most sensitive analyses were performed with a 90%-efficient HPGe gamma-ray detector, which is enclosed in a purged active/passive shield. Each sample was counted for one to six days in two orientations to yield more representative average activities for the sample. The non-standard geometries of the LDEF samples prompted the development of a novel calibration method, whereby the efficiency about the samples surfaces (measured with point sources) predicted the efficiency for the bulk sample.

  18. Gamma spectrometry of the minor bodies of the solar system

    SciTech Connect

    Surkov, Yu.A.; Moskaleva, L.P.; Manvelyan, O.S.

    1987-01-01

    The authors investigate the possibility of determining the elemental composition of the surfaces of minor bodies of the solar system (asteroids, the Martian satellites Phobos and Deimos, etc.) using spacecraft-based ..gamma..-spectrometry. The dependence of ..gamma..-photon flux on altitude above the body was calculated for body radii from 13 to 500 km. Estimates were made of the sensitivity of the determination of basic rock-forming elements with respect to changes in geometry of a factor of two, using ..gamma..-spectrometry with a 100 mm by 100 mm crystal of NaI(Tl). Finally, the time required to determine the stipulated characteristic ..gamma..-radiation of surface rocks with the given precision was derived as a function of altitude.

  19. High-resolution gamma-ray spectrometry in uranium exploration

    USGS Publications Warehouse

    Moxham, Robert M.; Tanner, Allan B.

    1977-01-01

    Sedimentary-type uranium deposits accumulate at favorable sites along a migration path which may be kilometers in length. Their source is a large volume of rock from which the uranium has been leached. The geochemical mobilities and half lives of uranium and its daughter products vary widely so that they are transported from the source rocks, at different rates, along the migration path to their ultimate site. The radioactive disequilibrium resulting from this process has been well documented in the immediate vicinity of ore deposits, and disequilibrium is commonly recorded on gamma-ray logs up the hydraulic gradient from uranium ore. Little is known about the state of secular equilibrium in the leached host rocks, which often represent the only part of the migration path that is at or near the surface and is thus most accessible to the exploration geophysicist. High-resolution gamma-ray spectrometry provides a means of investigating the disequilibrium associated with uranium leaching and migration. Direct measurement of uranium can be made by this method, and the equivalent weight percents can be determined for six of the seven daughter-product decay groups that characterize the state of radioactive equilibrium. The technique has been used quantitatively in laboratory studies, where the results compare favorably with radiochemical analyses; field experiments suggest that semi-quantitative data may be obtained at the outcrop.

  20. The Dortmund Low Background Facility - Low-background gamma ray spectrometry with an artificial overburden.

    PubMed

    Gastrich, Holger; Gößling, Claus; Klingenberg, Reiner; Kröninger, Kevin; Neddermann, Till; Nitsch, Christian; Quante, Thomas; Zuber, Kai

    2016-06-01

    The Dortmund Low Background Facility is an instrument for low-level gamma ray spectrometry with an artificial overburden of ten meters of water equivalent, an inner shielding, featuring a neutron absorber, and an active muon veto. An integral background count rate between 40keV and 2700keV of (2.528±0.004)counts/(kgmin) enables low-background gamma ray spectrometry with sensitivities in the range of some 10mBq/kg within a week of measurement time. PMID:27082973

  1. Low-resolution gamma-ray measurements of uranium enrichment

    SciTech Connect

    Sprinkle, J.K. Jr.; Christiansen, A.; Cole, R.; Collins, M.L.

    1996-11-01

    Facilities that process special nuclear material perform periodic inventories. In bulk facilities that process low-enriched uranium, these inventories and their audits are based primarily on weight and enrichment measurements. Enrichment measurements determine the {sup 211}U weight fraction of the uranium compound from the passive gamma-ray emissions of the sample. Both international inspectors and facility operators rely on the capability to make in-field gamma-ray measurements of uranium enrichment. These users require rapid, portable measurement capability. Some in-field measurements have been biased, forcing the inspectors to resort to high-resolution measurements or mass spectrometry to accomplish their goals.

  2. Development of isotope dilution gamma-ray spectrometry for plutonium analysis

    SciTech Connect

    Li, T.K.; Parker, J.L. ); Kuno, Y.; Sato, S.; Kurosawa, A.; Akiyama, T. )

    1991-01-01

    We are studying the feasibility of determining the plutonium concentration and isotopic distribution of highly radioactive, spent-fuel dissolver solutions by employing high-resolution gamma-ray spectrometry. The study involves gamma-ray plutonium isotopic analysis for both dissolver and spiked dissolver solution samples, after plutonium is eluted through an ion-exchange column and absorbed in a small resin bead bag. The spike is well characterized, dry plutonium containing {approximately}98% of {sup 239}Pu. By using measured isotopic information, the concentration of elemental plutonium in the dissolver solution can be determined. Both the plutonium concentration and the isotopic composition of the dissolver solution obtained from this study agree well with values obtained by traditional isotope dilution mass spectrometry (IDMS). Because it is rapid, easy to operate and maintain, and costs less, this new technique could be an alternative method to IDMS for input accountability and verification measurements in reprocessing plants. 7 refs., 4 figs., 4 tabs.

  3. Application of in-situ gamma spectrometry in the remediation of radioactively contaminated soil

    SciTech Connect

    Sutton, C.; Yesso, J.D.; Danahy, R.J.; Cox, T.

    1999-06-01

    The Fernald Environmental Management Project (FEMP) is a US Department of Energy site that is undergoing total remediation and closure. Most of the remediation effort entails massive excavation of soil for disposal, both offsite and onsite, at an engineered disposal facility. In-situ gamma spectrometry is routinely used to support soil excavation operations to accurately and quickly identify soil areas as being above or below regulatory remediation criteria. Two different in-situ gamma spectrometry systems are used. The first is a sodium iodide (NaI) detector mounted either on a tractor or a jogging stroller, depending on the terrain to be measured. The NaI system allows the collection of a gamma energy spectrum which can be analyzed to identify and quantify radioactive isotopes which are present within the detector`s viewing area. Each energy spectrum is tagged by location coordinates provided by an on-board global positioning system (GPS) to precisely locate elevated contamination areas. The second is a tripod-mounted, high purity germanium detector (HPGe) gamma spectrometry system that is functionally similar to the NaI system. The principal advantage of the HPGe is its superior resolution, which allows much more accurate identification and quantification of radionuclide contaminants in soils. In order to effectively utilize the data quality objective process with these systems, three quality assurance (QA) elements had to be performed.

  4. Gamma ray spectrometry of LDEF samples at SRS

    NASA Technical Reports Server (NTRS)

    Winn, Willard G.

    1991-01-01

    A total of 31 samples from Long Duration Exposure Facility (LDEF), including materials of Al, V, and steel trunnions were analyzed by ultralow level gamma spectrometry. The study quantified particle induced activations of Na-22, Sc-46, Cr-51, Mn-54, Co-56, Co-57, Co-58, and Co-60. The samples of trunnion sections exhibited increasing activity toward the outer end of the trunnion and decreasing activity toward its radial center. The trunnion sections did not include an end piece that collects noticeable Be-7 on its leading surface. No significant Be-7 was detected in the samples analyzed. The most sensitive analyses were performed with a 90 pct. efficient HPGe gamma ray detector, which is enclosed in a purged active/passive active shield.

  5. Measurement of. gamma gamma. psi final states in psi' decay

    SciTech Connect

    Himel, T.M.; Abrams, G.S.; Alam, M.S.; Blocker, C.A.; Boyarski, A.M.; Breidenbach, M.; Burke, D.L.; Carithers, W.C.; Chinowsky, W.; Coles, M.W.; Cooper, S.; Dieterle, W.E.; Dillon, J.B.; Dorenbosch, J.; Dorfan, J.M.; Eaton, M.W.; Feldman, G.J.; Franklin, M.E.B.; Gidal, G.; Goldhaber, G.; Hanson, G.; Hayes, K.G.; Hitlin, D.G.; Hollebeek, R.J.; Innes, W.R.; Jaros, J.A.; Jenni, P.; Johnson, A.D.; Kadyk, J.A.; Lankford, A.J.; Larsen, R.R.; Levi, M.E.; Lueth, V.; Millikan, R.E.; Nelson, M.E.; Pang, C.Y.; Patrick, J.F.; Perl, M.L.; Richter, B.; Roussarie, A.; Scharre, D.L.; Schindler, R.H.; Schwitters, R.F.; Siegrist, J.L.; Strait, J.; Taureg, H.; Tonutti, M.; Trilling, G.H.; Vella, E.N.; Vidal, R.A.; Videau, I.; Weiss, J.M.; Zaccone, H.

    1980-04-07

    The decay mode psi' ..-->.. ..gamma gamma..psi has been studied with the Mark-II detector at SPEAR. New measurements of branching ratios for decays of the type psi' ..-->.. ..gamma..chi, chi ..-->.. ..gamma..psi involving known chi states are presented. The existence of a chi state of mass near 3455 MeV/c/sup 2/ produced in this decay chain is not confirmed, and the upper limit (90% confidence level) of the product of branching ratios is measured to be 0.13%. A new decay mode, psi' ..-->.. ..pi../sup 0/psi, which violates isospin conservation is observed with branching ratio (0.15 +- 0.06)%.

  6. Determination of impurities in (124)I samples by high resolution gamma spectrometry.

    PubMed

    de Almeida, M C M; da Silva, R L; Delgado, J U; Poledna, R; de Araújo, M T F; Laranjeira, A S; de Veras, E; Braghirolli, A M S; dos Santos, G R; Lopes, R T

    2016-03-01

    (124)I is a radionuclide used in the diagnosis of tumors. The National Health Agency requires identification and activity measurement of impurities. Using gamma spectrometry with an efficiency calibrated high-purity germanium detector, impurities (125)I and (126)I in an (1)(24)I production sample were identified. Activity ratios of (125)I and (126)I to (124)I were approximately 0.5% and 98%, respectively. PMID:26653211

  7. Gamma ray spectrometry of LDEF samples at SRL

    NASA Technical Reports Server (NTRS)

    Winn, Willard G.

    1992-01-01

    A total of 31 samples from the Long Duration Exposure Facility (LDEF), including materials of aluminum, vanadium, and steel trunnions were analyzed by ultra-low-level gamma spectrometry. The study quantified particle induced activations of Na-22, Sc-46, Cr-51, Mn-54, Co-56, Co-57, Co-58, and Co-60. The samples of trunnion sections exhibited increasing activity toward the outer end of the trunnion and decreasing activity toward its radial center. The trunnion sections did not include end pieces, which were reported to collect noticeable Be-7 on their leading surfaces. No significant Be-7 was detected in the samples analyzed.

  8. Application of the Monte Carlo code DETEFF to efficiency calibrations for in situ gamma-ray spectrometry.

    PubMed

    Carrazana González, J; Cornejo Díaz, N; Jurado Vargas, M

    2012-05-01

    We studied the applicability of the Monte Carlo code DETEFF for the efficiency calibration of detectors for in situ gamma-ray spectrometry determinations of ground deposition activity levels. For this purpose, the code DETEFF was applied to a study case, and the calculated (137)Cs activity deposition levels at four sites were compared with published values obtained both by soil sampling and by in situ measurements. The (137)Cs ground deposition levels obtained with DETEFF were found to be equivalent to the results of the study case within the uncertainties involved. The code DETEFF could thus be used for the efficiency calibration of in situ gamma-ray spectrometry for the determination of ground deposition activity using the uniform slab model. It has the advantage of requiring far less simulation time than general Monte Carlo codes adapted for efficiency computation, which is essential for in situ gamma-ray spectrometry where the measurement configuration yields low detection efficiency. PMID:22336296

  9. Testing of regolith of celestial bolides with active neutron gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Vostrukhin, Andrey; Mitrofanov, Igor; Golovin, Dmitry; Litvak, Maxim; Sanin, Anton

    2015-04-01

    Current space instruments for studying planet's surface include gamma ray spectrometers that detect natural radioactive isotopes as well as gamma-rays induced in subsurface by galactic cosmic rays. When measuring from celestial body's surface, statistics and amount of detected elements can be dramatically increased with active methods, where soil exposed to artificial flux of particles. One good example is the Russian Dynamic Albedo of Neutron (DAN) instrument onboard Martian Science Laboratory mission (Curiosity rover) developed in 2005-2011. It is the first active neutron spectrometer flown to another planet as part of a landed mission to investigate subsurface water distribution and which has now successfully operated for more than two years on the Martian surface. Presentation describes a number of space instruments for different landers and rovers being developed in Russian Space Research Institute for studying Moon and Mars, as well as method of active neutron and gamma spectrometry overview.

  10. Use of Gamma Spectrometry Method for Environmental Monitoring in the area of NPP

    NASA Astrophysics Data System (ADS)

    Thinova, L.; Cechak, T.; Kluson, J.; Trojek, T.

    2006-05-01

    It is generally not possible to correctly determine the long and short term impact of human activity upon the environment, without thorough processing of data, obtained through monitoring. It was confirmed that such impact on the environment must be monitored over a long time period. The data obtained must be of high quality, an attribute assured by present state of scientific knowledge. One of the well established methods for monitoring atmospheric deposition of radionuclides in the environment is laboratory and in situ gamma spectrometry. With the aim to monitor an occurrence of a one-time escape or persistent release of fission products into the air, resulting from an operation of a nuclear plant, two types of monitoring are performed: i/ measurement of samples from the environment (Schreber moss, forest humus, pine bark, mushrooms and forest berries) using laboratory gamma spectrometry method in the range up to 3 MeV (those data are used for the trend analysis and for the construction of the contaminationmaps); ii/ in situ gama spectrometry for assessment dosimetry and spectrometry characteristic of photon-fields (those data are used for the dose rate calculation).

  11. Measurement of the gamma gamma* --> eta and gamma gamma* --> eta' transition form factors

    SciTech Connect

    del Amo Sanchez et al, P.

    2011-02-07

    We study the reactions e{sup +}e{sup -} {yields} e{sup +}e{sup -} {eta}{sup (/)} in the single-tag mode and measure the {gamma}{gamma}* {yields} {eta}{sup (/)} transition form factors in the momentum transfer range from 4 to 40 GeV{sup 2}. The analysis is based on 469 fb{sup -1} of integrated luminosity collected at PEP-II with the BABAR detector at e{sup +}e{sup -} center-of-mass energies near 10.6 GeV.

  12. Applications of gamma-ray spectrometry in the quantitative nondestructive assay of special nuclear materials

    SciTech Connect

    Sampson, T.E.; Parker, J.L.

    1990-04-16

    Nearly all applications of gamma-ray spectrometry in the quanitative assay of special nuclear materials can be grouped into five general categories. They are as follows: (1) Quanitative passive assay, of which transmission-corrected passive assay methods for measuring isotopic masses/concentrations are an important subset; (2) Enrichment measurements on infinitely thick'' samples for absolute determination of isotopic fractions/concentrations; (3) Measurements of isotopic ratios using relative detection efficiency principles resulting in absolute isotopic distributions without recourse to standards; (4) Absorption-edge densitometry measurements of elemental concentrations; and (5) X-ray fluorescence measurements of elemental concentrations. Careful and correct practice of these techniques can yield measurement accuracies in the range of 0.1% to 1.0% in favorable situations with measurement times generally in the range of 15 minutes to 1 hour. We present examples of these general categories with emphasis on those measurements and techniques exhibiting the best accuracy, as well as those which are not routinely practiced in many other applications of gamma-ray spectrometry. 20 refs., 6 fig.

  13. Uncertainty analysis of in-situ gamma spectrometry measurements of air cleaning filter cartridges and 200 L drums by a HPGe detector.

    PubMed

    Slaninka, Alojz; Slávik, Ondrej; Necas, Vladimír

    2010-01-01

    This work deals with most significant sources of uncertainty in determination of radionuclides massic activity in 200 L drums with radioactive waste (RAW) from decommissioning of nuclear power plant (NPP) A1 and operational air cleaning filters coming from different parts of NPP's ventilation system. It turned out that the most significant source of uncertainty is determination of photo peak detection efficiency, in particular measurement geometry. The detection efficiency of HPGe detector has been determined by calculation using ISOCS software (In Situ Object Counting System) and detector characteristics delivered by the manufacturer (LABSOCS). The detector efficiency is influenced by various factors like measurement geometry, deviation from standard geometry, environmental characteristics, sample properties (density, material composition), used collimator etc. Mentioned factors and their contributions to the uncertainty of detection efficiency and thus to the total uncertainty of massic activity determination have been individually evaluated in the paper. The main part of the work consists of evaluation of maximum uncertainty factor due to presence of hypothetical point source in measurement volume for both types of measurement geometry.

  14. Uncertainty analysis of in-situ gamma spectrometry measurements of air cleaning filter cartridges and 200 L drums by a HPGe detector.

    PubMed

    Slaninka, Alojz; Slávik, Ondrej; Necas, Vladimír

    2010-01-01

    This work deals with most significant sources of uncertainty in determination of radionuclides massic activity in 200 L drums with radioactive waste (RAW) from decommissioning of nuclear power plant (NPP) A1 and operational air cleaning filters coming from different parts of NPP's ventilation system. It turned out that the most significant source of uncertainty is determination of photo peak detection efficiency, in particular measurement geometry. The detection efficiency of HPGe detector has been determined by calculation using ISOCS software (In Situ Object Counting System) and detector characteristics delivered by the manufacturer (LABSOCS). The detector efficiency is influenced by various factors like measurement geometry, deviation from standard geometry, environmental characteristics, sample properties (density, material composition), used collimator etc. Mentioned factors and their contributions to the uncertainty of detection efficiency and thus to the total uncertainty of massic activity determination have been individually evaluated in the paper. The main part of the work consists of evaluation of maximum uncertainty factor due to presence of hypothetical point source in measurement volume for both types of measurement geometry. PMID:19945884

  15. Evaluation of radiological data of some saturated fatty acids using gamma ray spectrometry

    NASA Astrophysics Data System (ADS)

    Kore, Prashant S.; Pawar, Pravina P.; Palani Selvam, T.

    2016-02-01

    Radiological parameters such as mass attenuation coefficients (μm), total attenuation cross section (σtot), molar extinction coefficient (ε), mass energy absorption coefficient (μen/ρ) and effective electronic cross section (σt, el) of saturated fatty acids, namely butyric acid (C4H8O2), caproic acid (C6H12O2), enanthic acid (C7H14O2), caprylic acid (C8H16O2), pelargonic acid (C9H18O2) and valeric acid (C5H10O2) were measured using NaI(Tl)-based gamma spectrometry. Radioactive sources used in the study are 57Co, 133Ba, 137Cs, 54Mn, 60Co and 22Na. Gamma ray transmission method in a narrow beam good geometry set up was used in the study. The measured data were compared against Win-XCOM-based data. The agreement is within 1%.

  16. Comparison of LabSOCS and GESPECOR codes used in gamma-ray spectrometry.

    PubMed

    Done, L; Tugulan, L C; Gurau, D; Dragolici, F; Alexandru, C

    2016-03-01

    Two dedicated software packages -LabSOCS and GESPECOR- for efficiency evaluation in gamma-ray spectrometry, were compared for equivalence. The detection efficiency and the coincidence-summing corrections coefficients were calculated for a specific HPGe detector, for different sample parameters and energies typically encountered in environmental radioactivity measurements. The discrepancy between the results obtained with the two codes were acceptable for most of the applications. Furthermore, the deviations between the values of the standard sources/ reference materials activities from the certificate and the values obtained after Monte Carlo simulation were less than 8% for LabSOCS and 9% for GESPECOR. PMID:26625727

  17. Low Background Gamma-Ray Spectrometry in the 'Laboratoire Souterrain de Modane'

    SciTech Connect

    Hubert, Ph.; Hubert, F.

    2007-03-28

    Most of the underground experiments in physics and many studies in geology, biology or environmental sciences face a common requirement with the necessity of using experimental devices with ultra-low background radioactivity. Many developments involving many different techniques have been used in order to be able to measure extremely low levels of radioactivity in materials. This report will focus on low background gamma-ray spectrometry and will describe the work which has been carried out over the last fifteen years in the 'Laboratoire Souterrain de Modane' (LSM)

  18. Contribution of atmospherical radon to in-situ scintillation gamma spectrometry data.

    PubMed

    Klusoň, J; Thinová, L

    2011-08-01

    In-situ gamma spectrometry can be used for monitoring and determining natural and man-made radionuclide concentrations in the environment. The low detection limit of potential contaminants depends on the natural background variations, including variations in the atmospheric concentrations of radon and its decay products. The scintillation spectrometer response for atmospheric radon was simulated by the Monte Carlo method, and the results were compared with the experimental measurements over large water surfaces. The contributions of atmospheric radon to the natural background were assessed. PMID:21129988

  19. Thorium determination in intercomparison samples and in some Romanian building materials by gamma ray spectrometry.

    PubMed

    Pantelica, A; Georgescu, I I; Murariu-Magureanu, M D; Margaritescu, I; Cincu, E

    2001-01-01

    Thorium content in zircon sand, thorium ore and a thorium liquid sample (EU Laboratories Network Intercomparison), as well as in some Romanian building materials: sand, wood, tufa, asbestos-cement. cement mill dust, coal fly ash, bricks, and tile (28 samples) was deterimined by gamma ray spectrometry. For the building materials, 226Ra, 40K and 137Cs specific activities were also measured. The results were compared with the Romanian legal norms concerning the highest admissible levels for 232Th, 226Ra. and 40K radioactivity. and to Th, U, and K concentration values previously determined in our laboratory on similar types of samples.

  20. Comparison of digital signal processing modules in gamma-ray spectrometry.

    PubMed

    Lépy, Marie-Christine; Cissé, Ousmane Ibrahima; Pierre, Sylvie

    2014-05-01

    Commercial digital signal-processing modules have been tested for their applicability to gamma-ray spectrometry. The tests were based on the same n-type high purity germanium detector. The spectrum quality was studied in terms of energy resolution and peak area versus shaping parameters, using a Eu-152 point source. The stability of a reference peak count rate versus the total count rate was also examined. The reliability of the quantitative results is discussed for their use in measurement at the metrological level.

  1. An analysis of nuclear fuel burnup in the AGR-1 TRISO fuel experiment using gamma spectrometry, mass spectrometry, and computational simulation techniques

    DOE PAGES

    Harp, Jason M.; Demkowicz, Paul A.; Winston, Philip L.; Sterbentz, James W.

    2014-09-03

    AGR 1 was the first in a series of experiments designed to test US TRISO fuel under high temperature gas-cooled reactor irradiation conditions. This experiment was irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) and is currently undergoing post irradiation examination (PIE) at INL and Oak Ridge National Laboratory. One component of the AGR 1 PIE is the experimental evaluation of the burnup of the fuel by two separate techniques. Gamma spectrometry was used to non destructively evaluate the burnup of all 72 of the TRISO fuel compacts that comprised the AGR 1 experiment. Two methodsmore » for evaluating burnup by gamma spectrometry were developed, one based on the Cs 137 activity and the other based on the ratio of Cs 134 and Cs 137 activities. Burnup values determined from both methods compared well with the values predicted from simulations. The highest measured burnup was 20.1% FIMA for the direct method and 20.0% FIMA for the ratio method (compared to 19.56% FIMA from simulations). An advantage of the ratio method is that the burnup of the cylindrical fuel compacts can determined in small (2.5 mm) axial increments and an axial burnup profile can be produced. Destructive chemical analysis by inductively coupled mass spectrometry (ICP MS) was then performed on selected compacts that were representative of the expected range of fuel burnups in the experiment to compare with the burnup values determined by gamma spectrometry. The compacts analyzed by mass spectrometry had a burnup range of 19.3% FIMA to 10.7% FIMA. The mass spectrometry evaluation of burnup for the four compacts agreed well with the gamma spectrometry burnup evaluations and the expected burnup from simulation. For all four compacts analyzed by mass spectrometry, the maximum range in the three experimentally determined values and the predicted value was 6% or less. Furthermore, the results confirm the accuracy of the nondestructive burnup evaluation from gamma

  2. An analysis of nuclear fuel burnup in the AGR-1 TRISO fuel experiment using gamma spectrometry, mass spectrometry, and computational simulation techniques

    SciTech Connect

    Harp, Jason M.; Demkowicz, Paul A.; Winston, Philip L.; Sterbentz, James W.

    2014-09-03

    AGR 1 was the first in a series of experiments designed to test US TRISO fuel under high temperature gas-cooled reactor irradiation conditions. This experiment was irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) and is currently undergoing post irradiation examination (PIE) at INL and Oak Ridge National Laboratory. One component of the AGR 1 PIE is the experimental evaluation of the burnup of the fuel by two separate techniques. Gamma spectrometry was used to non destructively evaluate the burnup of all 72 of the TRISO fuel compacts that comprised the AGR 1 experiment. Two methods for evaluating burnup by gamma spectrometry were developed, one based on the Cs 137 activity and the other based on the ratio of Cs 134 and Cs 137 activities. Burnup values determined from both methods compared well with the values predicted from simulations. The highest measured burnup was 20.1% FIMA for the direct method and 20.0% FIMA for the ratio method (compared to 19.56% FIMA from simulations). An advantage of the ratio method is that the burnup of the cylindrical fuel compacts can determined in small (2.5 mm) axial increments and an axial burnup profile can be produced. Destructive chemical analysis by inductively coupled mass spectrometry (ICP MS) was then performed on selected compacts that were representative of the expected range of fuel burnups in the experiment to compare with the burnup values determined by gamma spectrometry. The compacts analyzed by mass spectrometry had a burnup range of 19.3% FIMA to 10.7% FIMA. The mass spectrometry evaluation of burnup for the four compacts agreed well with the gamma spectrometry burnup evaluations and the expected burnup from simulation. For all four compacts analyzed by mass spectrometry, the maximum range in the three experimentally determined values and the predicted value was 6% or less. Furthermore, the results confirm the accuracy of the nondestructive burnup evaluation from gamma spectrometry

  3. Gamma-ray spectrometry in the cascade area of a gas centrifuge enrichment plant

    SciTech Connect

    Lauppe, W.D.; Richter, B.; Stein, G.

    1985-01-01

    In the frame of the programme of the Federal Republic of Germany in support of the IAEA, measurements were performed in the SP4 gas centrifuge enrichment plant in Almelo, the Netherlands. The objective was the investigation of the applicability of non-destructive ..gamma..-spectrometry equipment - presently available to the IAEA - at uranium-hexafluoride cascade piping for the purpose of measuring the uranium enrichment. The measurement locations were chosen at the product pipework between the top of a cascade and the first valve, which is inside the cascade area. Taking account of the results of the Hexapartite Safeguards Project, the measurement method should be capable of giving a go/no go result on current and preceding production of high-enriched uranium. The paper gives a description of the acquired measurement method and evaluation. The measurement results are discussed and conclusions are drawn.

  4. A Case Study Correlating Innovative Gamma Ray Scanning Detection Systems Data to Surface Soil Gamma Spectrometry Results - 13580

    SciTech Connect

    Thompson, Shannon; Rodriguez, Rene; Billock, Paul; Lit, Peter

    2013-07-01

    HydroGeoLogic (HGL), Inc. completed a United States Environmental Protection Agency (USEPA) study to characterize radiological contamination at a site near Canoga Park, California. The characterized area contained 470 acres including the site of a prototype commercial nuclear reactor and other nuclear design, testing, and support operations from the 1950's until 1988 [1]. The site history included radiological releases during operation followed by D and D activities. The characterization was conducted under an accelerated schedule and the results will support the project remediation. The project has a rigorous cleanup to background agenda and does not allow for comparison to risk-based guidelines. To target soil sample locations, multiple lines of evidence were evaluated including a gamma radiation survey, geophysical surveys, historical site assessment, aerial photographs, and former worker interviews. Due to the time since production and decay, the primary gamma emitting radionuclide remaining is cesium-137 (Cs-137). The gamma ray survey covered diverse, rugged terrain using custom designed sodium iodide thallium-activated (NaI(Tl)) scintillation detection systems. The survey goals included attaining 100% ground surface coverage and detecting gamma radiation as sensitively as possible. The effectiveness of innovative gamma ray detection systems was tested by correlating field Cs-137 static count ratios to Cs-137 laboratory gamma spectrometry results. As a case study, the area encompassing the former location of the first nuclear power station in the U. S. was scanned, and second by second global positioning system (GPS)-linked gamma spectral data were evaluated by examining total count rate and nuclide-specific regions of interest. To compensate for Compton scattering from higher energy naturally occurring radionuclides (U-238, Th-232 and their progeny, and K-40), count rate ratios of anthropogenic nuclide-specific regions of interest to the total count rate were

  5. Automated gamma spectrometry and data analysis on radiometric neutron dosimeters

    SciTech Connect

    Matsumoto, W.Y.

    1983-01-01

    An automated gamma-ray spectrometry system was designed and implemented by the Westinghouse Hanford Company at the Hanford Engineering Development Laboratory (HEDL) to analyze radiometric neutron dosimeters. Unattended, automatic, 24 hour/day, 7 day/week operation with online data analysis and mainframe-computer compatible magnetic tape output are system features. The system was used to analyze most of the 4000-plus radiometric monitors (RM's) from extensive reactor characterization tests during startup and initial operation of th Fast Flux Test Facility (FFTF). The FFTF, operated by HEDL for the Department of Energy, incorporates a 400 MW(th) sodium-cooled fast reactor. Aumomated system hardware consists of a high purity germanium detector, a computerized multichannel analyzer data acquisition system (Nuclear Data, Inc. Model 6620) with two dual 2.5 Mbyte magnetic disk drives plus two 10.5 inch reel magnetic tape units for mass storage of programs/data and an automated Sample Changer-Positioner (ASC-P) run with a programmable controller. The ASC-P has a 200 sample capacity and 12 calibrated counting (analysis) positions ranging from 6 inches (15 cm) to more than 20 feet (6.1 m) from the detector. The system software was programmed in Fortran at HEDL, except for the Nuclear Data, Inc. Peak Search and Analysis Program and Disk Operating System (MIDAS+).

  6. Monitoring radioactive plumes by airborne gamma-ray spectrometry

    SciTech Connect

    Grasty, R.L.; Hovgaard, J.; Multala, J.

    1996-06-01

    Airborne gamma-ray spectrometer surveys using large volume sodium-iodide detectors are routinely flown throughout the world for mineral exploration and geological mapping. Techniques have now been developed to detect and map man-made sources of radiation. In Canada, airborne gamma-rays surveys have been flown around nuclear reactors to map {sup 41}Ar plumes from nuclear reactors and to calculate the dose rate at ground level. In May 1986, the Finnish Geological survey aircraft flew through a radioactive plume from the Chernobyl nuclear accident. As the aircraft flew through the plume, the aircraft became increasingly contaminated. By measuring the final aircraft contamination, the activity of the plume could be separated from the contamination due to the aircraft. Within 1 h of encountering the plume, the aircraft activity was comparable to the maximum levels found in the plume. From an analysis of the gamma-ray spectra, the concentration of {sup 131}I and {sup 140}La within the plume were calculated as a function of time.

  7. Indoor and outdoor in situ high-resolution gamma radiation measurements in urban areas of Cyprus.

    PubMed

    Svoukis, E; Tsertos, H

    2007-01-01

    In situ, high-resolution, gamma-ray spectrometry of a total number of 70 outdoor and 20 indoor representative measurements were performed in preselected, common locations of the main urban areas of Cyprus. Specific activities and gamma absorbed dose rates in air due to the naturally occurring radionuclides of (232)Th and (238)U series, and (40)K are determined and discussed. Effective dose rate to the Cyprus population due to terrestrial gamma radiation is derived directly from this work. The results obtained outdoors match very well with those derived previously by high-resolution gamma spectrometry of soil samples, which were collected from the main island bedrock surface. This implies that the construction and building materials in urban areas do not affect the external gamma dose rate; thus they are mostly of local origin. Finally, the indoor/outdoor gamma dose ratio was found to be 1.4 +/- 0.5. PMID:17065195

  8. Measurements of Gamma in BaBar

    SciTech Connect

    Marchiori, G.; /INFN, Pisa

    2006-08-30

    We report on the first measurements to the angle {gamma} of the Unitarity Triangle in B meson decays collected by the BABAR detector at the SLAC PEP-II asymmetric-energy B factory in the years 1999-2004.

  9. Dead time, pileup, and accurate gamma-ray spectrometry

    SciTech Connect

    Lindstrom, R.M.; Fleming, R.F.

    1995-12-31

    The accuracy of gamma-ray spectrometric measurements is ultimately limited by the precision of Poisson counting statistics. With careful attention to detail, all other sources of error in the ratio of activities of two sources of a radionuclide in small samples can be made insignificant, even when the statistical limit is well below one percent. An important source of error comes from the finite time required by the counting electronics to detect and process pulses. Dead-time losses (mostly in the analog-digital converter) are usually compensated very well by the pulse-height analyzer, but pileup losses (mostly in the amplifier) may not be. Errors of 10% or more may easily result. Several methods are available for detecting and correcting rate-related losses. These methods are sufficiently reliable and well understood that a decaying source can be measured with acceptably small errors even at count rates as high as tens of thousands per second.

  10. Waste Characterization Using Gamma Ray Spectrometry with Automated Efficiency Optimization - 13404

    SciTech Connect

    Bosko, A.; Venkataraman, R.; Bronson, F.L.; Ilie, G.; Russ, W.R.

    2013-07-01

    Gamma ray spectrometry using High Purity Germanium (HPGe) detectors is commonly employed in assaying radioactive waste streams from a variety of sources: nuclear power plants, Department of Energy (DOE) laboratories, medical facilities, decontamination and decommissioning activities etc. The radioactive material is typically packaged in boxes or drums (for e.g. B-25 boxes or 208 liter drums) and assayed to identify and quantify radionuclides. Depending on the origin of the waste stream, the radionuclides could be special nuclear materials (SNM), fission products, or activation products. Efficiency calibration of the measurement geometry is a critical step in the achieving accurate quantification of radionuclide content. Due to the large size of the waste items, it is impractical and expensive to manufacture gamma ray standard sources for performing a measurement based calibration. For well over a decade, mathematical efficiency methods such as those in Canberra's In Situ Object Counting System (ISOCS) have been successfully employed in the efficiency calibration of gamma based waste assay systems. In the traditional ISOCS based calibrations, the user provides input data such as the dimensions of the waste item, the average density and fill height of the matrix, and matrix composition. As in measurement based calibrations, the user typically defines a homogeneous matrix with a uniform distribution of radioactivity. Actual waste containers can be quite nonuniform, however. Such simplifying assumptions in the efficiency calibration could lead to a large Total Measurement Uncertainty (TMU), thus limiting the amount of waste that can be disposed of as intermediate or low activity level waste. To improve the accuracy of radionuclide quantification, and reduce the TMU, Canberra has developed the capability to optimize the efficiency calibration using the ISOCS method. The optimization is based on benchmarking the efficiency shape and magnitude to the data available in the

  11. Measurement of the gamma gamma* -> pi0 transition form factor

    SciTech Connect

    Aubert, B.

    2009-06-02

    We study the reaction e{sup +}e{sup -} {yields} e{sup +}e{sup -}{pi}{sup 0} in the single tag mode and measure the differential cross section d{sigma}/dQ{sup 2} and the {gamma}{gamma}* {yields} {pi}{sup 0} transition form factor in the mometum transfer range from 4 to 40 GeV{sup 2}. At Q{sup 2} > 10 GeV{sup 2} the measured form factor exceeds the asymptotic limit predicted by perturbative QCD. The analysis is based on 442 fb{sup -1} of integrated luminosity collected at PEP-II with the BABAR detector at e{sup +}e{sup -} center-of-mass energies near 10.6 GeV.

  12. Cosmic veto gamma-spectrometry for Comprehensive Nuclear-Test-Ban Treaty samples

    NASA Astrophysics Data System (ADS)

    Burnett, J. L.; Davies, A. V.

    2014-05-01

    The Comprehensive Nuclear-Test-Ban Treaty (CTBT) is supported by a global network of monitoring stations that perform high-resolution gamma-spectrometry on air filter samples for the identification of 85 radionuclides. At the UK CTBT Radionuclide Laboratory (GBL15), a novel cosmic veto gamma-spectrometer has been developed to improve the sensitivity of station measurements, providing a mean background reduction of 80.8% with mean MDA improvements of 45.6%. The CTBT laboratory requirement for a 140Ba MDA is achievable after 1.5 days counting compared to 5-7 days using conventional systems. The system consists of plastic scintillation plates that detect coincident cosmic-ray interactions within an HPGe gamma-spectrometer using the Canberra LynxTM multi-channel analyser. The detector is remotely configurable using a TCP/IP interface and requires no dedicated coincidence electronics. It would be especially useful in preventing false-positives at remote station locations (e.g. Halley, Antarctica) where sample transfer to certified laboratories is logistically difficult. The improved sensitivity has been demonstrated for a CTBT air filter sample collected after the Fukushima incident.

  13. The 124Sb activity standardization by gamma spectrometry for medical applications

    NASA Astrophysics Data System (ADS)

    de Almeida, M. C. M.; Iwahara, A.; Delgado, J. U.; Poledna, R.; da Silva, R. L.

    2010-07-01

    This work describes a metrological activity determination of 124Sb, which can be used as radiotracer, applying gamma spectrometry methods with hyper pure germanium detector and efficiency curves. This isotope with good activity and high radionuclidic purity is employed in the form of meglumine antimoniate (Glucantime) or sodium stibogluconate (Pentostam) to treat leishmaniasis. 124Sb is also applied in animal organ distribution studies to solve some questions in pharmacology. 124Sb decays by β-emission and it produces several photons (X and gamma rays) with energy varying from 27 to 2700 keV. Efficiency curves to measure point 124Sb solid sources were obtained from a 166mHo standard that is a multi-gamma reference source. These curves depend on radiation energy, sample geometry, photon attenuation, dead time and sample-detector position. Results for activity determination of 124Sb samples using efficiency curves and a high purity coaxial germanium detector were consistent in different counting geometries. Also uncertainties of about 2% ( k=2) were obtained.

  14. Fast-ion energy resolution by one-step reaction gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Salewski, M.; Nocente, M.; Gorini, G.; Jacobsen, A. S.; Kiptily, V. G.; Korsholm, S. B.; Leipold, F.; Madsen, J.; Moseev, D.; Nielsen, S. K.; Rasmussen, J.; Stejner, M.; Tardocchi, M.; Contributors, JET

    2016-04-01

    The spectral broadening of γ-rays from fusion plasmas can be measured in high-resolution gamma-ray spectrometry (GRS). We derive weight functions that determine the observable velocity space and quantify the velocity-space sensitivity of one-step reaction high-resolution GRS measurements in magnetized fusion plasmas. The weight functions suggest that GRS resolves the energies of fast ions directly without the need for tomographic inversion for selected one-step reactions at moderate plasma temperatures. The D(p,γ)3He reaction allows the best direct fast-ion energy resolution. We illustrate our general formalism using reactions with and without intrinsic broadening of the γ-rays for the GRS diagnostic at JET.

  15. Gamma-ray measurements of a 6-kilogram neptunium sphere

    SciTech Connect

    Moss, C. E.; Frankle, C. M.

    2002-01-01

    In order to better determine the properties of {sup 237}Np for criticality safety and nuclear nonproliferation, especially its critical mass, 6070-gram solid sphere was cast on 15 May 2001 in a hot cell. The casting sprue was cut off on a lathe and the casting ground to a final diameter of 8.29 cm. The sphere was enclosed in a spherical tungsten shell 0.523-cm thick to reduce the gamma-ray dose. The neptunium and the tungsten were doubly encapsulated in welded, spherical nickel shells, each 0.381-cm thick. The sprue material was analyzed by mass spectrometry. Here we report the results of the first gamma-ray measurements of this unique item.

  16. Neutron and Gamma-ray Measurements

    SciTech Connect

    Krasilnikov, Anatoly V.; Sasao, Mamiko; Kaschuck, Yuri A.; Kiptily, Vasily G.; Popovichev, Sergey V.; Nishitani, Takeo; Bertalot, Luciano

    2008-03-12

    Due to high neutron and gamma-ray yields and large size plasmas many future fusion reactor plasma parameters such as fusion power, fusion power density, ion temperature, fuel mixture, fast ion energy and spatial distributions can be well measured by various fusion product diagnostics. Neutron diagnostics provide information on fusion reaction rate, which indicates how close is the plasma to the ultimate goal of nuclear fusion and fusion power distribution in the plasma core, which is crucial for optimization of plasma breakeven and burn. Depending on the plasma conditions neutron and gamma-ray diagnostics can provide important information, namely about dynamics of fast ion energy and spatial distributions during neutral beam injection, ion cyclotron heating and generated by fast ions MHD instabilities. The influence of the fast particle population on the 2-D neutron source profile was clearly demonstrated in JET experiments. 2-D neutron and gamma-ray source measurements could be important for driven plasma heating profile optimization in fusion reactors. To meat the measurement requirements in ITER the planned set of neutron and gamma ray diagnostics includes radial and vertical neutron and gamma cameras, neutron flux monitors, neutron activation systems and neutron spectrometers. The necessity of using massive radiation shielding strongly influences the diagnostic designs in fusion reactor, determines angular fields of view of neutron and gamma-ray cameras and spectrometers and gives rise to unavoidable difficulties in the absolute calibration. The development, testing in existing tokomaks and a possible engineering integration of neuron and gamma-ray diagnostic systems into ITER are presented.

  17. Neutron and Gamma-ray Measurements

    NASA Astrophysics Data System (ADS)

    Krasilnikov, Anatoly V.; Sasao, Mamiko; Kaschuck, Yuri A.; Kiptily, Vasily G.; Nishitani, Takeo; Popovichev, Sergey V.; Bertalot, Luciano

    2008-03-01

    Due to high neutron and gamma-ray yields and large size plasmas many future fusion reactor plasma parameters such as fusion power, fusion power density, ion temperature, fuel mixture, fast ion energy and spatial distributions can be well measured by various fusion product diagnostics. Neutron diagnostics provide information on fusion reaction rate, which indicates how close is the plasma to the ultimate goal of nuclear fusion and fusion power distribution in the plasma core, which is crucial for optimization of plasma breakeven and burn. Depending on the plasma conditions neutron and gamma-ray diagnostics can provide important information, namely about dynamics of fast ion energy and spatial distributions during neutral beam injection, ion cyclotron heating and generated by fast ions MHD instabilities. The influence of the fast particle population on the 2-D neutron source profile was clearly demonstrated in JET experiments. 2-D neutron and gamma-ray source measurements could be important for driven plasma heating profile optimization in fusion reactors. To meat the measurement requirements in ITER the planned set of neutron and gamma ray diagnostics includes radial and vertical neutron and gamma cameras, neutron flux monitors, neutron activation systems and neutron spectrometers. The necessity of using massive radiation shielding strongly influences the diagnostic designs in fusion reactor, determines angular fields of view of neutron and gamma-ray cameras and spectrometers and gives rise to unavoidable difficulties in the absolute calibration. The development, testing in existing tokomaks and a possible engineering integration of neuron and gamma-ray diagnostic systems into ITER are presented.

  18. Disintegration rate and gamma ray emission probability per decay measurement of 123I.

    PubMed

    Koskinas, M F; Gishitomi, K C; Brito, A B; Yamazaki, I M; Dias, M S

    2012-09-01

    A series of (123)I measurements have been carried out in a 4π(e(A),X)-γ coincidence system. The experimental extrapolation curve was determined and compared to Monte Carlo simulation, performed by code ESQUEMA. From the slope of the experimental curve, the total conversion coefficient for the 159 keV total gamma transition, α(159), was determined. All radioactive sources were also measured in an HPGe spectrometry system, in order to determine the gamma-ray emission probability per decay for several gamma transitions. All uncertainties involved and their correlations were analyzed applying the covariance matrix methodology and the measured parameters were compared with those from the literature.

  19. Gamma radiation background measurements from Spacelab 2

    NASA Technical Reports Server (NTRS)

    Paciesas, William S.; Gregory, John C.; Fishman, Gerald J.

    1988-01-01

    A Nuclear Radiation Monitor incorporating a NaI(Tl) scintillation detector was flown as part of the verification flight instrumentation on the Spacelab 2 mission, July 29 to August 6, 1985. Gamma-ray spectra were measured with better than 20 s resolution throughout most of the mission in the energy range 0.1 to 30 MeV. Knowledge of the decay characteristics and the geomagnetic dependence of the counting rates enable measurement of the various components of the Spacelab gamma-ray background: prompt secondary radiation, Earth albedo, and delayed induced radioactivity. The status of the data analysis and present relevant examples of typical background behavior are covered.

  20. Gamma radiation background measurements from Spacelab 2

    NASA Technical Reports Server (NTRS)

    Paciesas, William S.; Gregory, John C.; Fishman, Gerald J.

    1989-01-01

    A Nuclear Radiation Monitor incorporating a NaI(Tl) scintillation detector was flown as part of the verification flight instrumentation on the Spacelab 2 mission, July 29 to August 6, 1985. Gamma-ray spectra were measured with better than 20 s resolution throughout most of the mission in the energy range 0.1 to 30 MeV. Knowledge of the decay characteristics and the geomagnetic dependence of the counting rates enable measurement of the various components of the Spacelab gamma-ray background: prompt secondary radiation, earth albedo, and delayed induced radioactivity. The status of the data analysis and present relevant examples of typical background behavior are covered.

  1. NMIS with Imaging and Gamma Ray Spectrometry for Pu, HEU, HE and Other Materials

    SciTech Connect

    Mihalczo, John T; Mullens, James Allen

    2012-03-01

    The Nuclear Material Identification System (NMIS) has been under development at ORNL and the National Nuclear Security Administration (NNSA) Y-12 National Security Complex since 1984. In the mid-1990s, what is now the US Department of Energy (DOE) Office of Nuclear Verification (ONV) realized that it was a useful technology for future arms control treaty applications and supported further development of the system. In 2004, fast-neutron imaging was incorporated into the system. In 2007, the ONV decided to develop a fieldable version of the system, designated as FNMIS, for potential use in future treaties. The FNMIS is being developed to be compatible with the eventual incorporation of gamma-ray spectrometry and an information barrier. This report addresses how and what attributes could be determined by the FNMIS system with gamma-ray spectrometry. The NMIS is a time-dependent coincidence system that incorporates tomographic imaging (including mapping of the fission sites) and gamma-ray spectrometry. It utilizes a small, lightweight (30 lb), portable deuterium-tritium (DT) neutron (14.1 MeV) generator (4 x 10{sup 7} neutrons/second) for active interrogation and can also perform passive interrogation. A high-purity germanium (HPGe) gamma-ray detector with multichannel analysis can be utilized in conjunction with the source for active interrogation or passively. The system uses proton recoil scintillators: 32 small 2.5 x 2.5 x 10.2-cm-thick plastic scintillators for imaging and at least two 2 x 2 arrays of 27 x 27 x 10-cm-thick plastic scintillators that detect induced fission radiation. The DT generator contains an alpha detector that time and directionally tags a fan beam of some of the neutrons emitted and subdivides it into pixels. A fast (1 GHz) time correlation processor measures the time-dependent coincidence among all detectors in the system. A computer-controlled scanner moves the small detectors and the source appropriately for scanning a target object for

  2. Cadium-Zinc-Telluride (CZT) Gamma Ray Spectrometry

    SciTech Connect

    William Quam

    2001-09-01

    This report describes CZT crystals and their use in large arrays for generation of gamma ray spectra. Laboratory spectra will be shown together with spectra accumulated by various battery powered portable instruments (see Appendix A). One of these portable instruments was specifically constructed to minimize power consumption and yet provide reasonable isotope identification capability. Detailed data will be presented covering gamma energy resolution, gamma peak shapes, system background, and detector efficiency. Nearly all data were taken with very small crystals of CZT; cubes 5 mm on a side. A few spectra will be presented from cylindrical crystals of about the same size (see Appendix A). The small crystal size leads to low counting rates and extended counting times for reliable isotope identification. We have addressed this problem by using arrays of CZT crystals, initially two crystals and, at present, arrays of eight crystals. Data will be shown relating spectral parameters for these two arrays. System MDA is one way of combining resolution, efficiency, and background that will enable direct comparison of various detector types for individual isotope identification. We have calculated the MDA for an early dual crystal array and the current eight crystal array. Data derived from each array will be presented. In addition, it is possible to extrapolate the MDA methodology to much larger arrays. A 32-crystal array is under construction and extrapolations to 256 and 1024 crystals are considered possible. Estimated MDA values for these larger arrays are also presented. Several 8-crystal arrays have been constructed and versions have been incorporated into portable instruments. Descriptions of these small instruments are given covering physical size, weight, and general configuration. These instruments have been tested for shock and temperature effects and data will be presented on the results of these tests. The MDA concept will also allow extrapolation to large

  3. Summary of gamma spectrometry on local air samples from 1985--1995

    SciTech Connect

    Winn, W.G.

    1997-04-02

    This report summarizes the 1985--1995 results of low-level HPGe gamma spectrometry analysis of high-volume air samples collected at the Aiken Airport, which is about 25 miles north of SRS. The author began analyzing these samples with new calibrations using the newly developed GRABGAM code in 1985. The air sample collections were terminated in 1995, as the facilities at the Aiken Airport were no longer available. Air sample measurements prior to 1985 were conducted with a different analysis system (and by others prior to 1984), and the data were not readily available. The report serves to closeout this phase of local NTS air sample studies, while documenting the capabilities and accomplishments. Hopefully, the information will guide other applications for this technology, both locally and elsewhere.

  4. Specific activity to H*(10) conversion coefficients for in situ gamma spectrometry.

    PubMed

    Lemercier, M; Gurriaran, R; Bouisset, P; Cagnat, X

    2008-01-01

    The typical situations found in in situ gamma spectrometry have been simulated by Monte Carlo techniques to obtain the energy spectra of the photon fluence rate existing at 1 m above ground. The main difficulty found with the model is its slow convergence. A method to speed up the calculation has been derived. The results of the model have been thoroughly tested against existing data. In a final stage, the specific activity to H*(10) conversion coefficients have been derived for the typical scenarios encountered in the in situ gamma spectrometry. PMID:17942441

  5. Efficiency transfer using the GEANT4 code of CERN for HPGe gamma spectrometry.

    PubMed

    Chagren, S; Ben Tekaya, M; Reguigui, N; Gharbi, F

    2016-01-01

    In this work we apply the GEANT4 code of CERN to calculate the peak efficiency in High Pure Germanium (HPGe) gamma spectrometry using three different procedures. The first is a direct calculation. The second corresponds to the usual case of efficiency transfer between two different configurations at constant emission energy assuming a reference point detection configuration and the third, a new procedure, consists on the transfer of the peak efficiency between two detection configurations emitting the gamma ray in different energies assuming a "virtual" reference point detection configuration. No pre-optimization of the detector geometrical characteristics was performed before the transfer to test the ability of the efficiency transfer to reduce the effect of the ignorance on their real magnitude on the quality of the transferred efficiency. The obtained and measured efficiencies were found in good agreement for the two investigated methods of efficiency transfer. The obtained agreement proves that Monte Carlo method and especially the GEANT4 code constitute an efficient tool to obtain accurate detection efficiency values. The second investigated efficiency transfer procedure is useful to calibrate the HPGe gamma detector for any emission energy value for a voluminous source using one point source detection efficiency emitting in a different energy as a reference efficiency. The calculations preformed in this work were applied to the measurement exercise of the EUROMET428 project. A measurement exercise where an evaluation of the full energy peak efficiencies in the energy range 60-2000 keV for a typical coaxial p-type HpGe detector and several types of source configuration: point sources located at various distances from the detector and a cylindrical box containing three matrices was performed. PMID:26623928

  6. Efficiency transfer using the GEANT4 code of CERN for HPGe gamma spectrometry.

    PubMed

    Chagren, S; Ben Tekaya, M; Reguigui, N; Gharbi, F

    2016-01-01

    In this work we apply the GEANT4 code of CERN to calculate the peak efficiency in High Pure Germanium (HPGe) gamma spectrometry using three different procedures. The first is a direct calculation. The second corresponds to the usual case of efficiency transfer between two different configurations at constant emission energy assuming a reference point detection configuration and the third, a new procedure, consists on the transfer of the peak efficiency between two detection configurations emitting the gamma ray in different energies assuming a "virtual" reference point detection configuration. No pre-optimization of the detector geometrical characteristics was performed before the transfer to test the ability of the efficiency transfer to reduce the effect of the ignorance on their real magnitude on the quality of the transferred efficiency. The obtained and measured efficiencies were found in good agreement for the two investigated methods of efficiency transfer. The obtained agreement proves that Monte Carlo method and especially the GEANT4 code constitute an efficient tool to obtain accurate detection efficiency values. The second investigated efficiency transfer procedure is useful to calibrate the HPGe gamma detector for any emission energy value for a voluminous source using one point source detection efficiency emitting in a different energy as a reference efficiency. The calculations preformed in this work were applied to the measurement exercise of the EUROMET428 project. A measurement exercise where an evaluation of the full energy peak efficiencies in the energy range 60-2000 keV for a typical coaxial p-type HpGe detector and several types of source configuration: point sources located at various distances from the detector and a cylindrical box containing three matrices was performed.

  7. X-ray fluorescence and gamma-ray spectrometry combined with multivariate analysis for topographic studies in agricultural soil.

    PubMed

    de Castilhos, Natara D B; Melquiades, Fábio L; Thomaz, Edivaldo L; Bastos, Rodrigo Oliveira

    2014-10-15

    Physical and chemical properties of soils play a major role in the evaluation of different geochemical signature, soil quality, discrimination of land use type, soil provenance and soil degradation. The objectives of the present study are the soil elemental characterization and soil differentiation in topographic sequence and depth, using Energy Dispersive X-Ray Fluorescence (EDXRF) as well as gamma-ray spectrometry data combined with Principal Component Analysis (PCA). The study area is an agricultural region of Boa Vista catchment which is located at Guamiranga municipality, Brazil. PCA analysis was performed with four different data sets: spectral data from EDXRF, spectral data from gamma-ray spectrometry, concentration values from EDXRF measurements and concentration values from gamma-ray spectrometry. All PCAs showed similar results, confirmed by hierarchical cluster analysis, allowing the data grouping into top, bottom and riparian zone samples, i.e. the samples were separated due to its landscape position. The two hillslopes present the same behavior independent of the land use history. There are distinctive and characteristic patterns in the analyzed soil. The methodologies presented are promising and could be used to infer significant information about the region to be studied.

  8. X-ray fluorescence and gamma-ray spectrometry combined with multivariate analysis for topographic studies in agricultural soil.

    PubMed

    de Castilhos, Natara D B; Melquiades, Fábio L; Thomaz, Edivaldo L; Bastos, Rodrigo Oliveira

    2014-10-15

    Physical and chemical properties of soils play a major role in the evaluation of different geochemical signature, soil quality, discrimination of land use type, soil provenance and soil degradation. The objectives of the present study are the soil elemental characterization and soil differentiation in topographic sequence and depth, using Energy Dispersive X-Ray Fluorescence (EDXRF) as well as gamma-ray spectrometry data combined with Principal Component Analysis (PCA). The study area is an agricultural region of Boa Vista catchment which is located at Guamiranga municipality, Brazil. PCA analysis was performed with four different data sets: spectral data from EDXRF, spectral data from gamma-ray spectrometry, concentration values from EDXRF measurements and concentration values from gamma-ray spectrometry. All PCAs showed similar results, confirmed by hierarchical cluster analysis, allowing the data grouping into top, bottom and riparian zone samples, i.e. the samples were separated due to its landscape position. The two hillslopes present the same behavior independent of the land use history. There are distinctive and characteristic patterns in the analyzed soil. The methodologies presented are promising and could be used to infer significant information about the region to be studied. PMID:25464179

  9. Pulser injection with subsequent removal for gamma-ray spectrometry

    DOEpatents

    Hartwell, Jack K.; Goodwin, Scott G.; Johnson, Larry O.; Killian, E. Wayne

    1990-01-01

    An improved system for gamma-ray spectroscopy characterized by an interface module that controls the injection of electronic pulses as well as separation logic that enables storage of pulser events in a region of the spectrum of a multichannel analyzer distinct from the region reserved for storage of gamma-ray events. The module accomplishes this by tagging pulser events (high or low) injected into the amplification circuitry, adding an offset to the events so identified at the time the events are at the output of the analog to digital converter, and storing such events in the upper portion of the spectrum stored in the multichannel analyzer. The module can be adapted for use with existing gamma-ray spectroscopy equipment to provide for automatic analyses of radioisotopes.

  10. Application of gamma-ray spectrometry in a NORM industry for its radiometrical characterization

    NASA Astrophysics Data System (ADS)

    Mantero, J.; Gázquez, M. J.; Hurtado, S.; Bolívar, J. P.; García-Tenorio, R.

    2015-11-01

    Industrial activities involving Naturally Occurring Radioactive Materials (NORM) are found among the most important industrial sectors worldwide as oil/gas facilities, metal production, phosphate Industry, zircon treatment, etc. being really significant the radioactive characterization of the materials involved in their production processes in order to assess the potential radiological risk for workers or natural environment. High resolution gamma spectrometry is a versatile non-destructive radiometric technique that makes simultaneous determination of several radionuclides possible with little sample preparation. However NORM samples cover a wide variety of densities and composition, as opposed to the standards used in gamma efficiency calibration, which are either water-based solutions or standard/reference sources of similar composition. For that reason self-absorption correction effects (especially in the low energy range) must be considered individually in every sample. In this work an experimental and a semi-empirical methodology of self-absorption correction were applied to NORM samples, and the obtained results compared critically, in order to establish the best practice in relation to the circumstances of an individual laboratory. This methodology was applied in samples coming from a TiO2 factory (NORM industry) located in the south-west of Spain where activity concentration of several radionuclides from the Uranium and Thorium series through the production process was measured. These results will be shown in this work.

  11. A simple gamma spectrometry method for evaluating the burnup of MTR-type HEU fuel elements

    NASA Astrophysics Data System (ADS)

    Makmal, T.; Aviv, O.; Gilad, E.

    2016-10-01

    A simple method for the evaluation of the burnup of a materials testing reactor (MTR) fuel element by gamma spectrometry is presented. The method was applied to a highly enriched uranium MTR nuclear fuel element that was irradiated in a 5 MW pool-type research reactor for a total period of 34 years. The experimental approach is based on in-situ measurements of the MTR fuel element in the reactor pool by a portable high-purity germanium detector located in a gamma cell. To corroborate the method, analytical calculations (based on the irradiation history of the fuel element) and computer simulations using a dedicated fuel cycle burnup code ORIGEN2 were performed. The burnup of the MTR fuel element was found to be 52.4±8.8%, which is in good agreement with the analytical calculations and the computer simulations. The method presented here is suitable for research reactors with either a regular or an irregular irradiation regime and for reactors with limited infrastructure and/or resources. In addition, its simplicity and the enhanced safety it confers may render this method suitable for IAEA inspectors in fuel element burnup assessments during on-site inspections.

  12. Gamma-ray spectrometry data collection and reduction by simple computing systems.

    PubMed

    Op de Beeck, J

    1975-12-01

    The review summarizes the present state of the involvement of relatively small computing devices in the collection and processing of gamma-ray spectrum data. An economic and utilitarian point of view has been chosen with regard to data collection in order to arrive at practically valuable conclusions in terms of feasibility of possible configurations with respect to their eventual application. A unified point of view has been adopted with regard to data processing by developing an information theoretical approach on a more or less intuitive level in an attempt to remove the largest part of the virtual disparity between the several processing methods described in the literature. A synoptical introduction to the most important mathematical methods has been incorporated, together with a detailed theoretical description of the concept gamma-ray spectrum. In accordance with modern requirements, the discussions are mainly oriented towards high-resolution semiconductor detector-type spectra. The critical evaluation of the processing methods reviewed is done with respect to a set of predefined criteria. Smoothing, peak detection, peak intensity determination, overlapping peak resolving and detection and upper limits are discussed in great detail. A preferred spectrum analysis method combining powerful data reduction properties with extreme simplicity and speed of operation is suggested. The general discussion is heavily oriented towards activation analysis application, but other disciplines making use of gamma-ray spectrometry will find the material presented equally useful. Final conclusions are given pointing to future developments and shifting their centre of gravity towards improving the quality of the measurements rather than expanding the use of tedious and sophisticated mathematical techniques requiring the limits of available computational power.

  13. On-line interrogation of pebble bed reactor fuel using passive gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Chen, Jianwei

    The Pebble Bed Reactor (PBR) is a helium-cooled, graphite-moderated high temperature nuclear power reactor. In addition to its inherently safe design, a unique feature of this reactor is its multipass fuel cycle in which graphite fuel pebbles (of varying enrichment) are randomly loaded and continuously circulated through the core until they reach their prescribed end-of-life burnup limit (˜80,000--100,000 MWD/MTU). Unlike the situation with conventional light water reactors (LWRs), depending solely on computational methods to perform in-core fuel management will be highly inaccurate. As a result, an on-line measurement approach becomes the only accurate method to assess whether a particular pebble has reached its end-of-life burnup limit. In this work, an investigation was performed to assess the feasibility of passive gamma-ray spectrometry assay as an approach for on-line interrogation of PBR fuel for the simultaneous determination of burnup and enrichment on a pebble-by-pebble basis. Due to the unavailability of irradiated or fresh pebbles, Monte Carlo simulations were used to study the gamma-ray spectra of the PBR fuel at various levels of burnup. A pebble depletion calculation was performed using the ORIGEN code, which yielded the gamma-ray source term that was introduced into the input of an MCNP simulation. The MCNP simulation assumed the use of a high-purity coaxial germanium detector. Due to the lack of one-group high temperature reactor cross sections for ORIGEN, a heterogeneous MCNP model was developed to describe a typical PBR core. Subsequently, the code MONTEBURNS was used to couple the MCNP model and ORIGEN. This approach allowed the development of the burnup-dependent, one-group spectral-averaged PBR cross sections to be used in the ORIGEN pebble depletion calculation. Based on the above studies, a relative approach for performing the measurements was established. The approach is based on using the relative activities of Np-239/I-132 in combination

  14. In situ gamma-ray spectrometry for environmental monitoring: a semi empirical calibration method.

    PubMed

    Boson, Jonas; Lidström, Kenneth; Nylén, Torbjörn; Agren, Göran; Johansson, Lennart

    2006-01-01

    In situ gamma spectrometry using high-purity germanium (HPGe) detectors is a frequently used method for the determination of radionuclide ground deposition levels. Such measurements do, however, require an efficiency calibration based on detector sensitivity and parameters such as soil density and vertical activity distribution. In this work, a novel expression is used for the detector efficiency, incorporating both the influence of photon energy and incidence angle. Detector-specific efficiency data are determined empirically. For the theoretical calculation of the photon fluence at the detector, a three-layer model of finite thickness is developed for the description of soil density and vertical activity distribution. In order to facilitate the calibration of in situ measurements, a PC program has been developed to enable rapid, on-site calculations of radionuclide ground deposition levels. The semi empirical calibration method was tested on in situ measurements with two different detectors, and the results show good agreement with results obtained from traditional soil sampling. PMID:16632586

  15. Total Absorption Gamma-ray Spectrometer (TAGS) Intensity Distributions from INL's Gamma-Ray Spectrometry Center

    DOE Data Explorer

    Greenwood, R. E.

    A 252Cf fission-product source and the INL on-line isotope separator were used to supply isotope-separated fission-product nuclides to a total absorption -ray spectrometer. This spectrometer consisted of a large (25.4-cm diameter x 30.5-cm long) NaI(Tl) detector with a 20.3-cm deep axial well in which is placed a 300-mm2 x 1.0-mm Si detector. The spectra from the NaI(Tl) detector are collected both in the singles mode and in coincidence with the B-events detected in the Si detector. Ideally, this detector would sum all the energy of the B- rays in each cascade following the population of daughter level by B- decay, so that the event could be directly associated with a particular daughter level. However, there are losses of energy from attenuation of the rays before they reach the detector, transmission of rays through the detector, escape of secondary photons from Compton scattering, escape of rays through the detector well, internal conversion, etc., and the measured spectra are thus more complicated than the ideal case and the analysis is more complex. Analysis methods have been developed to simulate all of these processes and thus provide a direct measure of the B- intensity distribution as a function of the excitation energy in the daughter nucleus. These data yield more accurate information on the B- distribution than conventional decay-scheme studies for complex decay schemes with large decay energies, because in the latter there are generally many unobserved and observed but unplaced rays. The TAGS data have been analyzed and published [R. E. Greenwood et al., Nucl Instr. and metho. A390(1997)] for 40 fission product-nuclides to determine the B- intensity distributions. [Copied from the TAGS page at http://www.inl.gov/gammaray/spectrometry/tags.shtml]. Those values are listed on this page for quick reference.

  16. Bioturbation coefficients of deep-sea sediments from the Peru Basin determined by gamma spectrometry of 210Pb exc

    NASA Astrophysics Data System (ADS)

    Suckow, Axel; Treppke, Ute; Wiedicke, Michael H.; Weber, Michael E.

    In the investigation of the impact of deep-sea mining on the ecosystem, the radioactive disequilibrium between 210Pb and 226Ra was studied in 16 surface sediment cores from the Peru Basin to obtain a quantitative measure of bioturbation. Gamma spectrometry was used as a fast, non-destructive, simultaneous assay of 210Pb and 226Ra. Buried manganese nodules and geochemical anomalies affect the depth profiles of these two radioisotopes. The calculated bioturbation coefficients show a high lateral variability. This made it impossible to detect a significant difference in bioturbation between two different study areas.

  17. A rapid dissolution procedure to aid initial nuclear forensics investigations of chemically refractory compounds and particles prior to gamma spectrometry.

    PubMed

    Reading, David G; Croudace, Ian W; Warwick, Phillip E; Britton, Richard

    2015-11-01

    A rapid and effective preparative procedure has been evaluated for the accurate determination of low-energy (40-200 keV) gamma-emitting radionuclides ((210)Pb, (234)Th, (226)Ra, (235)U) in uranium ores and uranium ore concentrates (UOCs) using high-resolution gamma ray spectrometry. The measurement of low-energy gamma photons is complicated in heterogeneous samples containing high-density mineral phases and in such situations activity concentrations will be underestimated. This is because attenuation corrections, calculated based on sample mean density, do not properly correct where dense grains are dispersed within a less dense matrix (analogous to a nugget effect). The current method overcomes these problems using a lithium tetraborate fusion that readily dissolves all components including high-density, self-attenuating minerals/compounds. This is the ideal method for dissolving complex, non-volatile components in soils, rocks, mineral concentrates, and other materials where density reduction is required. Lithium borate fusion avoids the need for theoretical efficiency corrections or measurement of matrix matched calibration standards. The resulting homogeneous quenched glass produced can be quickly dissolved in nitric acid producing low-density solutions that can be counted by gamma spectrometry. The effectiveness of the technique is demonstrated using uranium-bearing Certified Reference Materials and provides accurate activity concentration determinations compared to the underestimated activity concentrations derived from direct measurements of a bulk sample. The procedure offers an effective solution for initial nuclear forensic studies where complex refractory minerals or matrices exist. It is also significantly faster, safer and simpler than alternative approaches. PMID:26572834

  18. Uncertainty in HPGe detector calibrations for in situ gamma-ray spectrometry.

    PubMed

    Boson, Jonas; Johansson, Lennart; Ramebäck, Henrik; Agren, Göran

    2009-06-01

    Semi-empirical methods are often used for efficiency calibrations of in situ gamma-ray spectrometry measurements with high-purity germanium detectors. The intrinsic detector efficiency is experimentally determined for different photon energies and angles of incidence, and a suitable expression for the efficiency is fitted to empirical data. In this work, the combined standard uncertainty of such an efficiency function for two detectors was assessed. The uncertainties in individual efficiency measurements were found to be about 1.9 and 3.1% (with a coverage factor k = 1, i.e. with a confidence interval of about 68%) for the two detectors. The main contributions to these uncertainties were found to originate from uncertainties in source-to-detector distance, source activity and full-energy peak count rate. The standard uncertainties of the fitted functions were found to be somewhat higher than the uncertainty of individual data points, i.e. 5.2 and 8.1% (k = 1). With the introduction of a new expression for the detector efficiency, these uncertainties were reduced to 3.7 and 4.2%, i.e. with up to a factor of two. Note that this work only addresses the uncertainty in the determination of intrinsic detector efficiency. PMID:19429646

  19. 241Am (n,gamma) isomer ratio measurement

    SciTech Connect

    Bond, Evelyn M; Vieira, David J; Moody, Walter A; Slemmons, Alice K

    2011-01-05

    The objective of this project is to improve the accuracy of the {sup 242}Cm/{sup 241}Am radiochemistry ratio. We have performed an activation experiment to measure the {sup 241}Am(n,{gamma}) cross section leading to either the ground state of {sup 242g}Am (t{sub 1/2} = 16 hr) which decays to {sup 242}Cm (t{sub 1/2} = 163 d) or the long-lived isomer {sup 242m}Am (t{sub 1/2} = 141 yr). This experiment will develop a new set of americium cross section evaluations that can be used with a measured {sup 242}Cm/{sup 241}Am radiochemical measurement for nuclear forensic purposes. This measurement is necessary to interpret the {sup 242}Cm/{sup 241}Am ratio because a good measurement of this neutron capture isomer ratio for {sup 241}Am does not exist. The targets were prepared in 2007 from {sup 241}Am purified from LANL stocks. Gold was added to the purified {sup 241}Am as an internal neutron fluence monitor. These targets were placed into a holder, packaged, and shipped to Forschungszentrum Karlsruhe, where they were irradiated at their Van de Graff facility in February 2008. One target was irradiated with {approx}25 keV quasimonoenergetic neutrons produced by the {sup 7}Li(p,n) reaction for 3 days and a second target was also irradiated for 3 days with {approx}500 keV neutrons. Because it will be necessary to separate the {sup 242}Cm from the {sup 241}Am in order to measure the amount of {sup 242}Cm by alpha spectrometry, research into methods for americium/curium separations were conducted concurrently. We found that anion exchange chromatography in methanol/nitric acid solutions produced good separations that could be completed in one day resulting in a sample with no residue. The samples were returned from Germany in July 2009 and were counted by gamma spectrometry. Chemical separations have commenced on the blank sample. Each sample will be spiked with {sup 244}Cm, dissolved and digested in nitric acid solutions. One third of each sample will be processed at a time

  20. Baseline measurements of terrestrial gamma radioactivity at the CEBAF site

    SciTech Connect

    Wollenberg, H.A.; Smith, A.R.

    1991-10-01

    A survey of the gamma radiation background from terrestrial sources was conducted at the CEBAF site, Newport News, Virginia, on November 12--16, 1990, to provide a gamma radiation baseline for the site prior to the startup of the accelerator. The concentrations and distributions of the natural radioelements in exposed soil were measured, and the results of the measurements were converted into gamma-ray exposure rates. Concurrently, samples were collected for laboratory gamma spectral analyses.

  1. Advances in room-temperature solid-state gamma-ray spectrometry

    SciTech Connect

    Iwanczyk, J.S.

    1983-01-01

    This article presents a review and analysis of different concepts of gamma-ray spectrometry using room-temperature solid-state detectors. The classical approach involving the use of a charge-sensitive preamplifier and attempting to collect all the ionization charge produced by the gamma ray is analyzed and discussed in terms of the charge transport parameters of the most promising compound semiconductor materials. It is concluded that compound semiconductor detector materials having a large disparity between the ..mu.. tau products for electrons and holes (such as HgI/sub 2/ and CdTe) will have rather poor energy resolution if the classical method of spectrometry requiring full charge collection is employed. 30 references.

  2. Use of a Shielded High Resolution Gamma Spectrometry System to Segregate LLW from Contact Handleable ILW Containing Plutonium - 13046

    SciTech Connect

    Lester, Rosemary; Wilkins, Colin; Chard, Patrick; Jaederstroem, Henrik; LeBlanc, Paul; Mowry, Rick; MacDonald, Sanders; Gunn, William

    2013-07-01

    Dounreay Site Restoration Limited (DSRL) have a number of drums of solid waste that may contain Plutonium Contaminated Material. These are currently categorised as Contact Handleable Intermediate Level Waste (CHILW). A significant fraction of these drums potentially contain waste that is in the Low Level Waste (LLW) category. A Canberra Q2 shielded high resolution gamma spectrometry system is being used to quantify the total activity of drums that are potentially in the LLW category in order to segregate those that do contain LLW from CHILW drums and thus to minimise the total volume of waste in the higher category. Am-241 is being used as an indicator of the presence of plutonium in the waste from its strong 59.54 keV gamma-ray; a knowledge of the different waste streams from which the material originates allows a pessimistic waste 'fingerprint' to be used in order to determine an upper limit to the activities of the weak and non-gamma-emitting plutonium and associated radionuclides. This paper describes the main features of the high resolution gamma spectrometry system being used by DSRL to perform the segregation of CHILW and LLW and how it was configured and calibrated using the Canberra In-Situ Object Counting System (ISOCS). It also describes how potential LLW drums are selected for assay and how the system uses the existing waste stream fingerprint information to determine a reliable upper limit for the total activity present in each measured drum. Results from the initial on-site commissioning trials and the first measurements of waste drums using the new monitor are presented. (authors)

  3. The potential of gamma-ray spectrometry as supplementary information for mapping central European soils

    NASA Astrophysics Data System (ADS)

    Schuler, U.; Bock, M.; Baritz, R.; Willer, J.; Pickert, E.; Kardel, K.; Herrmann, L.

    2012-04-01

    Permanently updated soil maps are needed inter alia for the prediction of landslide hazards, flooding and drought effects, land degradation monitoring, and precision farming. Since comprehensive and intensive field mapping is not affordable, alternative mapping approaches are required. A promising tool, with quite unrecognised potential for modern soil science is gamma-ray spectrometry. As the radioelements potassium, thorium and uranium respond differently to soil forming processes, it should be possible to infer from their concentration on weathering status, and after calibration on soil properties and types. This paper aims to investigate the potential of airborne gamma spectrometry for mapping of central European soils and soil properties. The study was conducted for a test site in Southern Saxony, Germany, 140*85 km wide, representing diverse soil landscapes. Seven different petrographic training and validation areas were chosen each. To assess the potential of gamma-ray spectrometry as additional data layer, predictions were carried out (i) with and (ii) without radiometric data. The outputs were compared with independent soil information of the validation areas. Both prediction runs used the following predictors: elevation, slope, curvature, planform curvature, profile curvature, terrain ruggedness index, relative altitude, vertical distance above drainage network, wetness index, and convergence index. As additional predictor parent material derived from a reclassification of the official geological map (1:1M scale) was used. As radiometric properties potassium, thorium and uranium were used. The radiometric raster datasets were generated by universal kriging using relative altitude as covariate. Training and validation datasets were selected from a comprehensive dataset representing more than 14.000 point data. Point data include soil types and substrates, and for more than 800 sites soil profiles with analysed texture, pH, exchangeable cations, nutrients

  4. Detection of /sup 210/Pb in the lungs of smokers by in-vivo gamma spectrometry

    SciTech Connect

    Berger, C.D.; Lane, B.H.

    1982-09-01

    Since mainstream smoke is highly enriched in /sup 210/Pb, alpha radiation from inhaled cigarette smoke particles has been proposed as a cancer-producing agent in cigarette smokers. /sup 210/Po and /sup 210/Pb have been observed in tobacco, cigarette smoke and in the lungs of smokers. Since /sup 210/Pb is highly enriched in mainstream smoke, there have been estimates of yearly excesses of /sup 210/Pb in the lungs of one-pack-a-day smokers of 3 to 10 pCi (0.11 to 0.37 Bq). The ORNL Whole Body Counter was used to verify this estimate by the methodology of high-resolution, in vivo gamma spectrometry. Measurements were made on 113 adult male non-radiation workers who have either smoked at least one pack of cigarettes per day for at least five years, or have never smoked cigarettes. An analysis-of-variance table was generated based on the Pb-ratio for each individual which revealed that there was no statistically significant increase in the amount of /sup 210/Pb in the lungs of smokers over those of non-smokers. Sources of error are also discussed.

  5. Characterization of gamma irradiated petrolatum eye ointment base by headspace-gas chromatography-mass spectrometry.

    PubMed

    Hong, Lan; Altorfer, Hans

    2002-06-20

    The effects of gamma irradiation on petrolatum eye ointment base (EOB) and its ingredients (white petrolatum, liquid paraffin, and wool fat) were studied at different irradiation doses. Forty-one volatile radiolysis products were detected and identified by a combined system of headspace-gas chromatography-mass spectrometry (HS-GC-MS). The characteristics of the radiolysis products and the degradation pathway were discussed in each case, respectively. GC method demonstrates that the component distribution patterns of eye ointment as well as its individual ingredients have no differences before and after gamma irradiation. The influence of gamma treatment on EOB was quantitatively determined at 15, 25 and 50 kGy. The concentrations of the radiolysis products increase linearly with increasing doses. Both qualitative and quantitative data show that irradiated eye ointment is safe for human use.

  6. Measurement of borneol based on infrared spectrometry

    NASA Astrophysics Data System (ADS)

    Gu, Xiaoyu; Wang, Yan; Sun, Huili; Xu, Kexin

    2005-02-01

    The infrared spectrometry contains multiple information of the sample, and it is easy to be applied to on-line measurement. To Chinese medicine, this technology can improve the standard of quality control and accelerate the modernization course. In this paper, we investigate the spectral characteristics of borneol, an effective ingredient in many Chinese medicines. The following results are achieved. In middle infrared (MIR) region, utilizing the linear relationship between absorption and concentration, the concentration of borneol with relative error within 4.30% in the strongest absorption region (2950-2970 cm(-1)) is measured; in near infrared (NIR) region, the predicted concentrations of borneol are calculated by using partial least squares (PLS) regression analysis, in which the wavelengths are selected by genetic algorithm (GA) from the absorption bands of borneol in NIR region. The predicted relative error of calibration model is less than 2%. This result shows that PLS regression analysis combining genetic algorithm is a good method to improve prediction and reduce data in NIR region.

  7. Measuring Cosmological Parameters with Gamma Ray Bursts

    NASA Astrophysics Data System (ADS)

    Amati, Lorenzo; Della Valle, Massimo

    2013-12-01

    In a few dozen seconds, gamma ray bursts (GRBs) emit up to 1054 erg in terms of an equivalent isotropically radiated energy Eiso, so they can be observed up to z 10. Thus, these phenomena appear to be very promising tools to describe the expansion rate history of the universe. Here, we review the use of the Ep,i-Eiso correlation of GRBs to measure the cosmological density parameter ΩM. We show that the present data set of GRBs, coupled with the assumption that we live in a flat universe, can provide independent evidence, from other probes, that ΩM 0.3. We show that current (e.g. Swift, Fermi/GBM, Konus-WIND) and forthcoming gamma ray burst (GRB) experiments (e.g. CALET/GBM, SVOM, Lomonosov/UFFO, LOFT/WFM) will allow us to constrain ΩM with an accuracy comparable to that currently exhibited by Type Ia supernovae (SNe-Ia) and to study the properties of dark energy and their evolution with time.

  8. Calculating Measurement Uncertainties for Mass Spectrometry Data

    NASA Astrophysics Data System (ADS)

    Essex, R. M.; Goldberg, S. A.

    2006-12-01

    A complete and transparent characterization of measurement uncertainty is fundamentally important to the interpretation of analytical results. We have observed that the calculation and reporting of uncertainty estimates for isotopic measurement from a variety of analytical facilities are inconsistent, making it difficult to compare and evaluate data. Therefore, we recommend an approach to uncertainty estimation that has been adopted by both US national metrology facilities and is becoming widely accepted within the analytical community. This approach is outlined in the ISO "Guide to the Expression of Uncertainty in Measurement" (GUM). The GUM approach to uncertainty estimation includes four major steps: 1) Specify the measurand; 2) Identify uncertainty sources; 3) Quantify components by determining the standard uncertainty (u) for each component; and 4) Calculate combined standard uncertainty (u_c) by using established propagation laws to combine the various components. To obtain a desired confidence level, the combined standard uncertainty is multiplied by a coverage factor (k) to yield an expanded uncertainty (U). To be consistent with the GUM principles, it is also necessary create an uncertainty budget, which is a listing of all the components comprising the uncertainty and their relative contribution to the combined standard uncertainty. In mass spectrometry, Step 1 is normally the determination of an isotopic ratio for a particular element. Step 2 requires the identification of the many potential sources of measurement variability and bias including: gain, baseline, cup efficiency, Schottky noise, counting statistics, CRM uncertainties, yield calibrations, linearity calibrations, run conditions, and filament geometry. Then an equation expressing the relationship of all of the components to the measurement value must be written. To complete Step 3, these potential sources of uncertainty must be characterized (Type A or Type B) and quantified. This information

  9. In situ gamma-ray spectrometry in the environment using dose rate spectroscopy

    NASA Astrophysics Data System (ADS)

    Ji, Young-Yong; Kim, Chang-Jong; Chung, Kun Ho; Choi, Hee-Yeoul; Lee, Wanno; Kang, Mun Ja; Park, Sang Tae

    2016-02-01

    In order to expand the application of dose rate spectroscopy to the environment, in situ gamma-ray spectrometry was first conducted at a height of 1 m above the ground to calculate the ambient dose rate and individual dose rate at that height, as well as the radioactivity in the soil layer for the detected gamma nuclides from the dose rate spectroscopy. The reliable results could be obtained by introducing the angular correction factor to correct the G-factor with respect to incident photons distributed in a certain range of angles. The intercomparison results of radioactivity using ISOCS software, an analysis of a sample taken from the soil around a detector, and dose rate spectroscopy had a difference of <20% for 214Pb, 214Bi, 228Ac, 212Bi, 208Tl, and 40K, except for 212Pb with low-energy photons, that is, <300 keV. In addition, the drawback of using dose rate spectroscopy, that is, all gamma rays from a nuclide should be identified to accurately assess the individual dose rate, was overcome by adopting the concept of contribution ratio of the key gamma ray to the individual dose rate of a nuclide, so that it could be accurately calculated by identifying only a key gamma ray from a nuclide.

  10. Dating of sediments from four Swiss prealpine lakes with (210)Pb determined by gamma-spectrometry: progress and problems.

    PubMed

    Putyrskaya, V; Klemt, E; Röllin, S; Astner, M; Sahli, H

    2015-07-01

    In this paper the most important problems in dating lake sediments with unsupported (210)Pb are summarized and the progress in gamma-spectrometry of the unsupported (210)Pb is discussed. The main topics of these studies concern sediment samples preparation for gamma-spectrometry, measurement techniques and data analysis, as well as understanding of accumulation and sedimentation processes in lakes. The vertical distributions of artificial ((137)Cs, (241)Am, (239)Pu) and natural radionuclides ((40)K, (210,214)Pb, (214)Bi) as well as stable trace elements (Fe, Mn, Pb) in sediment cores from four Swiss lakes were used as examples for the interpretation, inter-comparison and validation of depth-age relations established by three (210)Pb-based models (CF-CSR, CRS and SIT). The identification of turbidite layers and the influence of the turbidity flows on the accuracy of sediment dating is demonstrated. Time-dependent mass sedimentation rates in lakes Brienz, Thun, Biel and Lucerne are discussed and compared with published data.

  11. Precision of gamma-ray measurements of the effective specific power and effective {sup 240}Pu fraction of plutonium

    SciTech Connect

    Sampson, T.E.

    1992-05-01

    This paper uses gamma-ray spectrometry data from replicate measurements on 40 plutonium-bearing samples to examine the repeatability of the effective {sup 240}Pu fraction ({sup 240}Pu{sub eff}) and the effective specific power (P{sub eff}) calculated from the isotopic distribution analyzed with gamma-ray spectrometry codes. The measurements were used to identify the error component arising from repeatability in the determination of the isotopic composition of plutonium in the sample and the contribution of the error component to the uncertainty in total plutonium mass measurements from neutron coincidence counting ({sup 240}Pu{sub eff}) and calorimetry (P{sub eff}). The 40 samples had {sup 240}Pu{sub eff} percentages ranging from 2 to 39% and P{sub eff} values ranging from 2 to 16 mW/g Pu. Four different gamma-ray spectrometry codes (FRAM, MGA, Blue Box, and PUJRC) were used to analyze the data (not all samples were analyzed with each code). All analyses showed that the % relative standard deviation of P{sub eff} was smaller than that of {sup 240}Pu{sub eff}. This result coupled with a cursory examination of uncertainties in coincidence counting of well-characterized samples and water-bath calorimetry errors for the same types of samples lead to the conclusion that smaller uncertainties will be present in the total plutonium mass determined by the combination of calorimetry/gamma-ray spectrometry than in the mass determined by coincidence counting/gamma-ray spectrometry. An additional examination of the biases arising from the {sup 240}Pu correlation used in the gamma-ray spectrometry codes also supported this conclusion. 17 refs.

  12. Fluence Evaluations For Applications of In Situ Gamma-Ray Spectrometry in Non-Flat Terrain

    SciTech Connect

    Miller, Kevin M.

    1999-02-28

    Evaluations of gamma-ray fluence are made for source geometries that depart from the flat ground geometry that is used in standard applications of in situ spectrometry. Geometries considered include uniform source distributions for soil mounds on top of flat terrain, cylindrical wells, and rectangular trenches. The results indicate that scaling the standard fluence values for flat terrain by the ratio of solid angle subtended by the soil to 2π leads to fluence estimates that are accurate to within a few percent. Practical applications of in situ spectrometry in non-flat terrain also appears to be simplified by the fact that the angular correction factor for a typical coaxial detector in these geometries may typically be about the same as that computed for flat ground.

  13. A broadband gamma-ray spectrometry using novel unfolding algorithms for characterization of laser wakefield-generated betatron radiation

    NASA Astrophysics Data System (ADS)

    Jeon, Jong Ho; Nakajima, Kazuhisa; Kim, Hyung Taek; Rhee, Yong Joo; Pathak, Vishwa Bandhu; Cho, Myung Hoon; Shin, Jung Hun; Yoo, Byung Ju; Hojbota, Calin; Jo, Sung Ha; Shin, Kang Woo; Sung, Jae Hee; Lee, Seung Ku; Cho, Byeoung Ick; Choi, Il Woo; Nam, Chang Hee

    2015-12-01

    We present a high-flux, broadband gamma-ray spectrometry capable of characterizing the betatron radiation spectrum over the photon energy range from 10 keV to 20 MeV with respect to the peak photon energy, spectral bandwidth, and unique discrimination from background radiations, using a differential filtering spectrometer and the unfolding procedure based on the Monte Carlo code GEANT4. These properties are experimentally verified by measuring betatron radiation from a cm-scale laser wakefield accelerator (LWFA) driven by a 1-PW laser, using a differential filtering spectrometer consisting of a 15-filter and image plate stack. The gamma-ray spectra were derived by unfolding the photostimulated luminescence (PSL) values recorded on the image plates, using the spectrometer response matrix modeled with the Monte Carlo code GEANT4. The accuracy of unfolded betatron radiation spectra was assessed by unfolding the test PSL data simulated with GEANT4, showing an ambiguity of less than 20% and clear discrimination from the background radiation with less than 10%. The spectral analysis of betatron radiation from laser wakefield-accelerated electron beams with energies up to 3 GeV revealed radiation spectra characterized by synchrotron radiation with the critical photon energy up to 7 MeV. The gamma-ray spectrometer and unfolding method presented here facilitate an in-depth understanding of betatron radiation from LWFA process and a novel radiation source of high-quality photon beams in the MeV regime.

  14. A broadband gamma-ray spectrometry using novel unfolding algorithms for characterization of laser wakefield-generated betatron radiation

    SciTech Connect

    Jeon, Jong Ho Nakajima, Kazuhisa Pathak, Vishwa Bandhu; Cho, Myung Hoon; Yoo, Byung Ju; Shin, Kang Woo; Kim, Hyung Taek; Sung, Jae Hee; Lee, Seung Ku; Choi, Il Woo; Rhee, Yong Joo; Shin, Jung Hun; Jo, Sung Ha; Hojbota, Calin; Cho, Byeoung Ick; Nam, Chang Hee

    2015-12-15

    We present a high-flux, broadband gamma-ray spectrometry capable of characterizing the betatron radiation spectrum over the photon energy range from 10 keV to 20 MeV with respect to the peak photon energy, spectral bandwidth, and unique discrimination from background radiations, using a differential filtering spectrometer and the unfolding procedure based on the Monte Carlo code GEANT4. These properties are experimentally verified by measuring betatron radiation from a cm-scale laser wakefield accelerator (LWFA) driven by a 1-PW laser, using a differential filtering spectrometer consisting of a 15-filter and image plate stack. The gamma-ray spectra were derived by unfolding the photostimulated luminescence (PSL) values recorded on the image plates, using the spectrometer response matrix modeled with the Monte Carlo code GEANT4. The accuracy of unfolded betatron radiation spectra was assessed by unfolding the test PSL data simulated with GEANT4, showing an ambiguity of less than 20% and clear discrimination from the background radiation with less than 10%. The spectral analysis of betatron radiation from laser wakefield-accelerated electron beams with energies up to 3 GeV revealed radiation spectra characterized by synchrotron radiation with the critical photon energy up to 7 MeV. The gamma-ray spectrometer and unfolding method presented here facilitate an in-depth understanding of betatron radiation from LWFA process and a novel radiation source of high-quality photon beams in the MeV regime.

  15. Low level activity determination by means of gamma spectrometry with respect to the natural background fluctuation.

    PubMed

    Dragounová, Lenka; Rulík, Petr

    2013-11-01

    The determination of low level activities of natural radionuclides from the uranium and thorium series by gamma-spectrometry faces the problem of proper natural background subtraction. Background fluctuation can cause differences in activity determination. Also the minimum detectable activity (MDA) of natural and artificial radionuclides can be influenced by background fluctuation. In this paper, results of the background fluctuation of shielded HPGe detectors with relative efficiency of 50-150% are presented together with the assessment of its influence on the determination of natural and artificial radionuclides.

  16. Nuclear chemistry of returned lunar samples: Nuclide analysis by gamma-ray spectrometry

    NASA Technical Reports Server (NTRS)

    Okelley, G. D.

    1975-01-01

    Primordial and cosmogenic radionuclide concentrations are determined nondestructively by gamma-ray spectrometry in soil and rock samples from the returned Apollo 17 sample collection from Taurus-Littrow and Descartes. Geochemical evidence in support of field geology speculation concerning layering of the subfloor basalt flows is demonstrated along with a possible correlation of magmatic fractionation of K/U as a function of depth. The pattern of radionuclide concentrations observed in these samples is distinct due to proton bombardment by the intense solar flares of August 4-9, 1972. Such radionuclide determinations are used in determining lunar sample orientation and characterizing solar flare activity.

  17. Novel Beta-Gamma Coincidence Measurements Using Phoswich Detectors

    SciTech Connect

    Ely, James H.; Aalseth, Craig E.; Hayes, James C.; Heimbigner, Tom R.; McIntyre, Justin I.; Miley, Harry S.; Panisko, Mark E.; Ripplinger, Mike D.

    2003-09-30

    The PNNL has developed an Automated Radio-xenon Sampler/Analyzer (ARSA) for the CTBT to measure four radio-xenon isotopes using a beta-gamma coincidence counting detector. A novel method to measure beta-gamma coincidences using a phoswich detector with state-of-the-art pulse shape discrimination techniqueses has been investigated.

  18. Gamma astrometric measurement experiment -science and implementation

    NASA Astrophysics Data System (ADS)

    Gai, Mario; Vecchiato, Alberto; Lattanzi, Mario G.; Ligori, Sebastiano; Loreggia, Davide; Fineschi, Silvano

    GAME (Gamma Astrometric Measurement Experiment) is a mission concept taking advantage of astronomical techniques for high precision measurements of interest to Fundamental Physics, and in particular the γ parameter of the Parameterized Post-Newtonian formulation of gravi-tation theories modifying the General Relativity. A space based telescope, looking close to the Solar limb thanks to coronagraphic techniques, may implement astrometric measurements sim-ilar to those performed in the solar eclipse of 1919, when Dyson, Eddington and collaborators measured for the first time the gravitational bending of light. Simulations show that the final accuracy of GAME can reach the 10-7 level. GAME will be a decisive experiment for the understanding of gravity physics, cosmology and the Universe evolution. The observations leading to Dark Matter (e.g. galaxy rotation curves) and Dark Energy (accelerated expansion of the Universe) might be explained with a modified version of General Relativity, e.g. in which the curvature invariant R is no longer constant as in Einstein's equations, i.e. the f (R) gravity theories. A 10-7 level determination of γ will provide stringent constraints on acceptable theories. Also, high precision astrometry makes accessible other appealing measurements, e.g. the light deflection induced by the quadrupole moment of giant planets, like Jupiter or Saturn, and, by high precision determination of the orbits of Mercury and high elongation asteroids, the PPN parameter β. GAME may also carry out measurements on selected astrophysical targets, e.g. nearby, bright stars known to host companions with minimum masses in the planetary/brown dwarf regime, and orbital radii in the 3-7 AU range, which are observed by no other present or planned campaigns. GAME, also thanks to high-cadence, high-precision photometry on transit-ing exoplanet systems, will thus improve on our understanding of the actual mass distribution and multiplicity of sub-stellar companions

  19. Inelastic cross sections from gamma-ray measurements

    SciTech Connect

    Nelson, Ronald Owen

    2010-12-06

    Measurements of gamma rays following neutron induced reactions have been studied with the Germanium Array for Neutron-induced Excitations (GEANIE) at the Los Alamos Neutron Science Center (LANSCE) for many years. Gamma-ray excitation functions and coincidence studies provide insight into nuclear reaction mechanisms as well as expanding our knowledge of energy levels and gamma-rays. Samples studied with Ge detectors at LANSCE range from Be to Pu. Fe, Cr and Ti have been considered for use as reference cross sections. An overview of the measurements and efforts to create a reliable neutron-induced gamma-ray reference cross section will be presented.

  20. Measurement of Disintegration Rates and Absolute {gamma}-ray Intensities

    SciTech Connect

    DeVries, Daniel J.; Griffin, Henry C.

    2006-03-13

    The majority of practical radioactive materials decay by modes that include {gamma}-ray emission. For questions of 'how much' or 'how pure', one must know the absolute intensities of the major radiations. We are using liquid scintillation counting (LSC) to measurements of disintegration rates, coupled with {gamma}-ray spectroscopy to measure absolute {gamma}-ray emission probabilities. Described is a study of the 227Th chain yielding absolute {gamma}-ray intensities with {approx}0.5% accuracy and information on LSC efficiencies.

  1. Measurements of Branching Fractions for B+ -> rho+ gamma, B0 -> rho0 gamma, and B0 -> omega gamma

    SciTech Connect

    Aubert, B

    2008-08-15

    The authors present branching fraction measurements for the radiative decays B{sup +} {yields} {rho}{sup +}{gamma}, B{sup 0} {yields} {rho}{sup 0}{gamma}, and B{sup 0} {yields} {omega}{gamma}. The analysis is based on a data sample of 465 million B{bar B} events collected with the BABAR detector at the PEP-II asymmetric-energy B Factory located at the Stanford Linear Accelerator Center (SLAC). They find {Beta}(B{sup +} {yields} {rho}{sup +}{gamma}) = (1.20{sub -0.37}{sup +0.42} {+-} 0.20) x 10{sup -6}, {Beta}(B{sup 0} {yields} {rho}{sup 0}{gamma}) = (0.97{sub -0.22}{sup +0.24} {+-} 0.06) x 10{sup -6}, and a 90% C.L. upper limit {Beta}(B{sup 0} {yields} {omega}{gamma}) < 0.9 x 10{sup -6}, where the first error is statistical and the second is systematic. They also measure the isospin-violating quantity {Lambda}(B{sup +} {yields} {rho}{sup +}{gamma})/2{Lambda}(B{sup 0} {yields} {rho}{sup 0}{gamma}) - 1 = -0.43{sub -0.22}{sup +0.25} {+-} 0.10.

  2. Measurements of cross sections relevant to. gamma. -ray line astronomy

    SciTech Connect

    Lesko, K.T.; Norman, E.B.; Larimer, R.M.; Crane, S.G.

    1986-06-01

    Gamma-ray production cross sections have been measured for the ..gamma..-ray lines which are mostly strongly excited in the proton bombardment of C, O, Mg, Si, and Fe targets of natural isotopic composition. High resolution germanium detectors were used to collect ..gamma..-ray spectra at proton bombarding energies of 20, 30, 33, 40 and 50 MeV. 6 refs., 6 figs.

  3. Isotope ratio measurements by secondary ion mass spectrometry (SIMS) and glow discharge mass spectrometry (GDMS)

    NASA Astrophysics Data System (ADS)

    Betti, Maria

    2005-04-01

    The basic principles of secondary ion mass spectrometry and glow discharge mass spectrometry have been shortly revisited. The applications of both techniques as exploited for the isotope ratio measurements in several matrices have been reviewed. Emphasis has been given to research fields in expansions such as solar system studies, medicine, biology, environment and nuclear forensic. The characteristics of the two techniques are discussed in terms of sensitivity and methodology of quantification. Considerations on the different detection possibilities in SIMS are also presented.

  4. The measurement of gamma ray induced heating in a mixed neutron and gamma ray environment

    SciTech Connect

    Chiu, H.K.

    1991-10-01

    The problem of measuring the gamma heating in a mixed DT neutron and gamma ray environment was explored. A new detector technique was developed to make this measurement. Gamma heating measurements were made in a low-Z assembly irradiated with 14-Mev neutrons and (n, n{prime}) gammas produced by a Texas Nuclear Model 9400 neutron generator. Heating measurements were made in the mid-line of the lattice using a proportional counter operating in the Continuously-varied Bias-voltage Acquisition mode. The neutron-induced signal was separated from the gamma-induced signal by exploiting the signal rise-time differences inherent to radiations of different linear energy transfer coefficient, which are observable in a proportional counter. The operating limits of this measurement technique were explored by varying the counter position in the low-Z lattice, hence changing the irradiation spectrum observed. The experiment was modelled numerically to help interpret the measured results. The transport of neutrons and gamma rays in the assembly was modelled using the one- dimensional radiation transport code ANISN/PC. The cross-section set used for these calculations was derived from the ENDF/B-V library using the code MC{sup 2}-2 for the case of DT neutrons slowing down in a low-Z material. The calculated neutron and gamma spectra in the slab and the relevant mass-stopping powers were used to construct weighting factors which relate the energy deposition in the counter fill-gas to that in the counter wall and in the surrounding material. The gamma energy deposition at various positions in the lattice is estimated by applying these weighting factors to the measured gamma energy deposition in the counter at those locations.

  5. Laser ablation inductively coupled plasma mass spectrometry measurement of isotope ratios in depleted uranium contaminated soils.

    PubMed

    Seltzer, Michael D

    2003-09-01

    Laser ablation of pressed soil pellets was examined as a means of direct sample introduction to enable inductively coupled plasma mass spectrometry (ICP-MS) screening of soils for residual depleted uranium (DU) contamination. Differentiation between depleted uranium, an anthropogenic contaminant, and naturally occurring uranium was accomplished on the basis of measured 235U/238U isotope ratios. The amount of sample preparation required for laser ablation is considerably less than that typically required for aqueous sample introduction. The amount of hazardous laboratory waste generated is diminished accordingly. During the present investigation, 235U/238U isotope ratios measured for field samples were in good agreement with those derived from gamma spectrometry measurements. However, substantial compensation was required to mitigate the effects of impaired pulse counting attributed to sample inhomogeneity and sporadic introduction of uranium analyte into the plasma.

  6. Laser ablation inductively coupled plasma mass spectrometry measurement of isotope ratios in depleted uranium contaminated soils.

    PubMed

    Seltzer, Michael D

    2003-09-01

    Laser ablation of pressed soil pellets was examined as a means of direct sample introduction to enable inductively coupled plasma mass spectrometry (ICP-MS) screening of soils for residual depleted uranium (DU) contamination. Differentiation between depleted uranium, an anthropogenic contaminant, and naturally occurring uranium was accomplished on the basis of measured 235U/238U isotope ratios. The amount of sample preparation required for laser ablation is considerably less than that typically required for aqueous sample introduction. The amount of hazardous laboratory waste generated is diminished accordingly. During the present investigation, 235U/238U isotope ratios measured for field samples were in good agreement with those derived from gamma spectrometry measurements. However, substantial compensation was required to mitigate the effects of impaired pulse counting attributed to sample inhomogeneity and sporadic introduction of uranium analyte into the plasma. PMID:14611049

  7. In-situ ground gamma spectrometry — an effective tool for geological mapping (the Male Karpaty Mts., Slovakia)

    NASA Astrophysics Data System (ADS)

    Mojzeš, Andrej; Porubčanová, Barbara

    2016-06-01

    This contribution presents the results of profile in-situ gamma spectrometry measurements that sought to determine the content of natural radionuclides 40K, 238U and 232Th in a near surface horizon of rocks, their weathering cover and soils in the area of the Malé Karpaty Mts. It is widely established that the exploration of radioactivity of bedrocks and cover rocks can be a very effective and useful tool for both geological mapping, for identifying deposits of mineral resources, and even addressing the issues of structural and tectonic geology. This assertion is equally confirmed by the ground gamma spectrometry measurements carried out as part of this case study on larger scales, seeking more detailed geological structure solutions. The results obtained provide a welcome addition to an already existing database, which monitors the content of naturally occurring radionuclides individually for every rock lithotype of the Western Carpathians, by elaborating on the data collected by previous research and by updating this database for any future needs. The presented results confirmed the low to medium radioactivity levels of rocks and soils in the studied area. The highest values were detected in granitoids and metamorfic phyllitic rocks of the Malé Karpaty Mts. core; the lowest values were detected in carbonates, arenaceous sediments and, above all, amphibolite bodies. In this way, the presented results of the interpreted profile (P5) confirm the model of local geological structure as represented on the most up-to-date edition of the geological map of the Male Karpaty Mts. (Polak et al. 2011).

  8. On the accuracy of gamma spectrometric isotope ratio measurements of uranium

    NASA Astrophysics Data System (ADS)

    Ramebäck, H.; Lagerkvist, P.; Holmgren, S.; Jonsson, S.; Sandström, B.; Tovedal, A.; Vesterlund, A.; Vidmar, T.; Kastlander, J.

    2016-04-01

    The isotopic composition of uranium was measured using high resolution gamma spectrometry. Two acid solutions and two samples in the form of UO2 pellets were measured. The measurements were done in close geometries, i.e. directly on the endcap of the high purity germanium detector (HPGe). Applying no corrections for count losses due to true coincidence summing (TCS) resulted in up to about 40% deviation in the abundance of 235U from the results obtained with mass spectrometry. However, after correction for TCS, excellent agreement was achieved between the results obtained using two different measurement methods, or a certified value. Moreover, after corrections, the fitted relative response curves correlated excellently with simulated responses, for the different geometries, of the HPGe detector.

  9. Measuring the charged pion polarizability in the gamma gamma -> pi+pi- reaction

    SciTech Connect

    Lawrence, David W.; Miskimen, Rory A.; Mushkarenkov, Alexander Nikolaevich; Smith, Elton S.

    2013-08-01

    Development has begun of a new experiment to measure the charged pion polarizability $\\alpha_{\\pi}-\\beta_{\\pi}$. The charged pion polarizability ranks among the most important tests of low-energy QCD presently unresolved by experiment. Analogous to precision measurements of $\\pi^{\\circ}\\rightarrow\\gamma\\gamma$ that test the intrinsic odd-parity (anomalous) sector of QCD, the pion polarizability tests the intrinsic even-parity sector of QCD. The measurement will be performed using the $\\gamma\\gamma\\rightarrow\\pi^{+{}}\\pi^{-{}}$ cross section accessed via the Primakoff mechanism on nuclear targets using the GlueX detector in Hall D at Jefferson Lab. The linearly polarized photon source in Hall-D will be utilized to separate the Primakoff cross-section from coherent $\\rho^{\\circ}$ production.

  10. Investigation of Failed TRISO Fuel Assay Using Gamma-Ray Spectrometry

    NASA Astrophysics Data System (ADS)

    Harp, Jason Michael

    TRISO microsphere fuel is the fundamental fuel unit for Very High Temperature Reactors (VHTR). A single TRISO particle consists of an inner kernel of Uranium Oxycarbide surrounded by layers of pyrolytic carbon and silicon carbide. The silicon carbide serves as the primary barrier to the release of fission products into the core. If the silicon carbide layer fails, fission gas, especially Kr and Xe, will begin to escape the failed particle. In order to understand the behavior of TRISO fuel under in-core conditions, a series of experiments is being conducted by Idaho National Lab at the Advanced Test Reactor. AGR-1 is the first of these experiments. It will measure fission product release due to failed TRISO particles. Simulations of this experiment have been conducted at North Carolina State University to develop a method for the analysis of the results of the experiment. The ATR core was simulated using the Monte Carlo code MCNP to calculate the expected neutron energy spectrum for the AGR-1 experimental test train. This spectrum was used to create one-group cross sections for implementation in ORIGEN calculations of the amount of activity produced in the experiment. Several theoretical models have been developed to describe the phenomenon of gas release. While each model is based on similar physics, different models contain unique features that distinguish them from one another. These Release to Birth (R/B) models are developed and applied to the activity found in the ORIGEN calculations to create expected release activities. The release activity is used to create gamma-ray spectra that are representative of the different R/B models. Expected R/B due to a model can be calculated for comparison to the experiment with knowledge of the number of failed particles in the spectra. The comparison of measured to predicted R/B ratios gives insight into the physics of release and also helps validate specific models. Direct comparison is possible, but many of the

  11. Analysis of spectra from portable handheld gamma-ray spectrometry for terrain comparative assessment.

    PubMed

    Dias, Flávio; Lima, Marco; Sanjurjo-Sánchez, Jorge; Alves, Carlos

    2016-04-01

    Geological characteristics can have impacts on societal development by, e.g., geotechnical issues and radiological hazard levels. Due to urban sprawl, there is an increasing need for detailed geological assessment. In this work are analysed data from portable handheld gamma-ray spectra (K, eU and eTh) obtained in granitic and Silurian metaclastic outcrops as well as in an profile, roughly N-S, on soil covered terrains transecting a mapped contact between these rock types (the profile's northern extremity is at locations mapped as granite). Estimations from gamma-ray spectra were studied by univariate and multivariate analyses. K, eU and eTh values were higher on granite in relation to Silurian metaclastic rocks. The northern extremity of the profile showed clearly higher contents of eTh and this contrast was supported by univariate statistical tools (normality plot and Wilk-Shapiro test; boxplots). A ternary plot with the contribution of the elements to gamma-ray absorbed dose showed the separation of granite from Silurian metaclastic rocks with the former being nearer the eTh vertex. The points in the northern extremity of the profile are nearer the eTh vertex than the other points on the profile. These visual suggestions were supported by hierarchical cluster analysis, which was able to differentiate between granite and metaclastic outcrops and separate portions of the profile located on different terrains. Portable gamma-ray spectrometry showed, hence, the potential to distinguish granite and metaclastic terrains at a scale useful for engineering works. These results can also be useful for a first comparative zoning of radiological hazards (which are higher for granite). PMID:26867098

  12. Analysis of spectra from portable handheld gamma-ray spectrometry for terrain comparative assessment.

    PubMed

    Dias, Flávio; Lima, Marco; Sanjurjo-Sánchez, Jorge; Alves, Carlos

    2016-04-01

    Geological characteristics can have impacts on societal development by, e.g., geotechnical issues and radiological hazard levels. Due to urban sprawl, there is an increasing need for detailed geological assessment. In this work are analysed data from portable handheld gamma-ray spectra (K, eU and eTh) obtained in granitic and Silurian metaclastic outcrops as well as in an profile, roughly N-S, on soil covered terrains transecting a mapped contact between these rock types (the profile's northern extremity is at locations mapped as granite). Estimations from gamma-ray spectra were studied by univariate and multivariate analyses. K, eU and eTh values were higher on granite in relation to Silurian metaclastic rocks. The northern extremity of the profile showed clearly higher contents of eTh and this contrast was supported by univariate statistical tools (normality plot and Wilk-Shapiro test; boxplots). A ternary plot with the contribution of the elements to gamma-ray absorbed dose showed the separation of granite from Silurian metaclastic rocks with the former being nearer the eTh vertex. The points in the northern extremity of the profile are nearer the eTh vertex than the other points on the profile. These visual suggestions were supported by hierarchical cluster analysis, which was able to differentiate between granite and metaclastic outcrops and separate portions of the profile located on different terrains. Portable gamma-ray spectrometry showed, hence, the potential to distinguish granite and metaclastic terrains at a scale useful for engineering works. These results can also be useful for a first comparative zoning of radiological hazards (which are higher for granite).

  13. Radiological Mapping of the Alkaline Intrusive Complex of Jombo, South Coastal Kenya by In-Situ Gamma-Ray Spectrometry

    NASA Astrophysics Data System (ADS)

    Kaniu, Ian; Darby, Iain G.; Kalambuka Angeyo, Hudson

    2016-04-01

    Carbonatites and alkaline intrusive complexes are rich in a variety of mineral deposits such as rare earth elements (REEs), including Nb, Zr and Mn. These are often associated with U and Th bearing minerals, including monazite, samarskite and pyrochlore. Mining waste resulting from mineral processing activities can be highly radioactive and therefore poses a risk to human health and environment. The Jombo complex located in Kenya's south coastal region is potentially one of the richest sources of Nb and REEs in the world. It consists of the main intrusion at Jombo hill, three associated satellite intrusions at Mrima, Kiruku and Nguluku hills, and several dykes. The complex is highly heterogeneous with regard to its geological formation as it is characterized by alkaline igneous rocks and carbonatites which also influence its radio-ecological dynamics. In-situ gamma spectrometry offers a low-cost, rapid and spatially representative radioactivity estimate across a range of landscapes compared to conventional radiometric techniques. In this work, a wide ranging radiological survey was conducted in the Jombo complex as follow up on previous studies[1,2], to determine radiation exposure levels and source distributions, and perform radiological risk assessments. The in-situ measurements were carried out using a 2.0 l NaI(Tl) PGIS-2 portable detector from Pico Envirotec Inc integrated with GPS, deployed for ground (back-pack) and vehicular gamma-ray spectrometry. Preliminary results of radiological distribution and mapping will be presented. [1] Patel, J. P. (1991). Discovery and Innovation, 3(3): 31-35. [2] Kebwaro, J. M. et. al. (2011). J. Phys. Sci., 6(13): 3105-3110.

  14. Perspectives of the GAMMA-400 space observatory for high-energy gamma rays and cosmic rays measurements

    NASA Astrophysics Data System (ADS)

    Topchiev, N. P.; Galper, A. M.; Bonvicini, V.; Adriani, O.; Aptekar, R. L.; Arkhangelskaja, I. V.; Arkhangelskiy, A. I.; Bakaldin, A. V.; Bergstrom, L.; Berti, E.; Bigongiari, G.; Bobkov, S. G.; Boezio, M.; Bogomolov, E. A.; Bonechi, S.; Bongi, M.; Bottai, S.; Castellini, G.; Cattaneo, P. W.; Cumani, P.; Dalkarov, O. D.; Dedenko, G. L.; De Donato, C.; Dogiel, V. A.; Finetti, N.; Gorbunov, M. S.; Gusakov, Yu V.; Hnatyk, B. I.; Kadilin, V. V.; Kaplin, V. A.; Kaplun, A. A.; Kheymits, M. D.; Korepanov, V. E.; Larsson, J.; Leonov, A. A.; Loginov, V. A.; Longo, F.; Maestro, P.; Marrocchesi, P. S.; Men'shenin, A. L.; Mikhailov, V. V.; Mocchiutti, E.; Moiseev, A. A.; Mori, N.; Moskalenko, I. V.; Naumov, P. Yu; Papini, P.; Pearce, M.; Picozza, P.; Rappoldi, A.; Ricciarini, S.; Runtso, M. F.; Ryde, F.; Serdin, O. V.; Sparvoli, R.; Spillantini, P.; Stozhkov, Yu I.; Suchkov, S. I.; Taraskin, A. A.; Tavani, M.; Tiberio, A.; Tyurin, E. M.; Ulanov, M. V.; Vacchi, A.; Vannuccini, E.; Vasilyev, G. I.; Yurkin, Yu T.; Zampa, N.; Zirakashvili, V. N.; Zverev, V. G.

    2016-02-01

    The GAMMA-400 gamma-ray telescope is intended to measure the fluxes of gamma-rays and cosmic-ray electrons and positrons in the energy range from 100 MeV to several TeV. Such measurements concern the following scientific tasks: investigation of point sources of gamma-rays, studies of the energy spectra of Galactic and extragalactic diffuse emission, studies of gamma-ray bursts and gamma-ray emission from the Sun, as well as high precision measurements of spectra of high-energy electrons and positrons. Also the GAMMA- 400 instrument provides the possibility for protons and nuclei measurements up to knee. But the main goal for the GAMMA-400 mission is to perform a sensitive search for signatures of dark matter particles in high-energy gamma-ray emission. To fulfill these measurements the GAMMA-400 gamma-ray telescope possesses unique physical characteristics in comparison with previous and present experiments. The major advantage of the GAMMA-400 instrument is excellent angular and energy resolution for gamma-rays above 10 GeV. The GAMMA-400 experiment will be installed onboard of the Navigator space platform, manufactured by the NPO Lavochkin Association. The expected orbit will be a highly elliptical orbit (with apogee 300.000 km and perigee 500 km) with 7 days orbital period. An important profit of such an orbit is the fact that the full sky coverage will always be available for gamma ray astronomy.

  15. Gamma-ray dosimetry measurements of the Little Boy replica

    SciTech Connect

    Plassmann, E.A.; Pederson, R.A.

    1984-01-01

    We present the current status of our gamma-ray dosimetry results for the Little Boy replica. Both Geiger-Mueller and thermoluminescent detectors were used in the measurements. Future work is needed to test assumptions made in data analysis.

  16. Steady-state differential calorimeter measures gamma heating in reactor

    NASA Technical Reports Server (NTRS)

    Herbst, D.; Talboy, J. H.

    1968-01-01

    Steady-state differential calorimeter, which displays good accuracy and reproducibility of results, is used to measure gamma heating in a reactor environment. The calorimeter has a long life expectancy since it is virtually unharmed by the reactor environment.

  17. Gamma spectrometry and chemical characterization of ceramic seeds with samarium-153 and holmium-166 for brachytherapy proposal.

    PubMed

    Valente, Eduardo S; Campos, Tarcísio P R

    2010-12-01

    Ceramic seeds were synthesized by the sol-gel technique with Si:Sm:Ca and Si:Ho:Ca. One set of seeds was irradiated in the TRIGA type nuclear reactor IPR-R1 and submitted to instrumental neutron activation analysis (INAA), K(0) method, to determine mass percentage concentration of natural samarium and holmium in the seed as well as to determine all existing radionuclides and their activities. Attention was paid to discrimination of Si-31, Ca-40, Ca-45, Ca-47, Ca-49, Sm-145, Sm-155, Sm-153 and Ho-166. A second sample was submitted to atomic emission spectrometry (ICP-AES) also to determine samarium and holmium concentrations in weight. A third sample was submitted to X-ray fluorescence spectrometry to qualitatively determine chemical composition. The measured activity was due to Sm-153 and Ho-166 with a well-characterized gamma spectrum. The X-ray fluorescence spectrum demonstrated that there is no discrepancy in seed composition. The maximum ranges in the water of beta particles from Sm-153 and Ho-166 decay were evaluated, as well as the dose rate and total dose delivered within the volume delimited by the range of the beta particles. The results are relevant for investigation of the viability of producing Sm-153 and Ho-166 radioactive seeds for use in brachytherapy.

  18. TLD measurements of gamma heating in heavy elements.

    NASA Technical Reports Server (NTRS)

    Reilly, H. J.; Robinson, R. A.; Peters, L. E., Jr.

    1971-01-01

    Measurements and calculations of gamma heating in polyethylene and lead containers were done and compared. The objective was to provide a workable method of getting good values for gamma heating in in-pile experiments containing materials of high atomic numbers. It was inferred that a combination of thermoluminescent dosimeter measurements, using Bragg-Gray theory, with photon transport calculations using the ANISN computer program, would meet this objective.

  19. Characterisation of imperial college reactor centre legacy waste using gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Shuhaimi, Alif Imran Mohd

    2016-01-01

    Waste characterisation is a principal component in waste management strategy. The characterisation includes identification of chemical, physical and radiochemical parameters of radioactive waste. Failure to determine specific waste properties may result in sentencing waste packages which are not compliant with the regulation of long term storage or disposal. This project involved measurement of intensity and energy of gamma photons which may be emitted by radioactive waste generated during decommissioning of Imperial College Reactor Centre (ICRC). The measurement will use High Purity Germanium (HPGe) as Gamma-ray detector and ISOTOPIC-32 V4.1 as analyser. In order to ensure the measurements provide reliable results, two quality control (QC) measurements using difference matrices have been conducted. The results from QC measurements were used to determine the accuracy of the ISOTOPIC software.

  20. Measurement of the {sup 157}Gd(n,{gamma}) reaction with the DANCE {gamma} calorimeter array

    SciTech Connect

    Chyzh, A.; Dashdorj, D.; Baramsai, B.; Mitchell, G. E.; Walker, C. L.; Becker, J. A.; Parker, W.; Wu, C. Y.; Becvar, F.; Kroll, J.; Krticka, M.; Bredeweg, T. A.; Couture, A.; Haight, R. C.; Jandel, M.; O'Donnell, J. M.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.

    2011-07-15

    The {sup 157}Gd(n,{gamma}) reaction was measured with the DANCE {gamma} calorimeter (consisting of 160 BaF{sub 2} scintillation detectors) at the Los Alamos Neutron Science Center. The multiplicity distributions of the {gamma} decay were used to determine the resonance spins up to E{sub n}=300 eV. The {gamma}-ray energy spectra for different multiplicities were measured for the s-wave resonances. The shapes of these spectra were compared with simulations based on the use of the DICEBOX statistical model code. Simulations showed that the scissors mode is required not only for the ground-state transitions but also for transitions between excited states.

  1. Isotopic composition analysis and age dating of uranium samples by high resolution gamma ray spectrometry

    NASA Astrophysics Data System (ADS)

    Apostol, A. I.; Pantelica, A.; Sima, O.; Fugaru, V.

    2016-09-01

    Non-destructive methods were applied to determine the isotopic composition and the time elapsed since last chemical purification of nine uranium samples. The applied methods are based on measuring gamma and X radiations of uranium samples by high resolution low energy gamma spectrometric system with planar high purity germanium detector and low background gamma spectrometric system with coaxial high purity germanium detector. The "Multigroup γ-ray Analysis Method for Uranium" (MGAU) code was used for the precise determination of samples' isotopic composition. The age of the samples was determined from the isotopic ratio 214Bi/234U. This ratio was calculated from the analyzed spectra of each uranium sample, using relative detection efficiency. Special attention is paid to the coincidence summing corrections that have to be taken into account when performing this type of analysis. In addition, an alternative approach for the age determination using full energy peak efficiencies obtained by Monte Carlo simulations with the GESPECOR code is described.

  2. A convenient method for discriminating between natural and depleted uranium by gamma-ray spectrometry.

    PubMed

    Shoji, M; Hamajima, Y; Takatsuka, K; Honoki, H; Nakajima, T; Kondo, T; Nakanishi, T

    2001-08-01

    A convenient method for discriminating between natural and depleted uranium reagent was developed by measuring and analyzing the gamma-ray spectra of some reagents with no standard source. The counting rates (R) of photoelectric peaks of gamma-rays from nuclides with the same radioactivity divided by their emission probability (B) are expressed as a function of gamma-ray energy. The radioactivities of 234Th and 234mPa and 21.72 times that of 235U are equal to the radioactivity of 235U in natural uranium. Therefore, the plot of 21.72-fold R/B for 235U should be on a curve fitted to the points for 234Th and 234mPa in natural uranium. Depleted uranium with a 235U isotopic composition of less than 0.68% could be discriminated from natural uranium in the case of a reagent containing 4.0 g of uranium.

  3. A convenient method for discriminating between natural and depleted uranium by gamma-ray spectrometry.

    PubMed

    Shoji, M; Hamajima, Y; Takatsuka, K; Honoki, H; Nakajima, T; Kondo, T; Nakanishi, T

    2001-08-01

    A convenient method for discriminating between natural and depleted uranium reagent was developed by measuring and analyzing the gamma-ray spectra of some reagents with no standard source. The counting rates (R) of photoelectric peaks of gamma-rays from nuclides with the same radioactivity divided by their emission probability (B) are expressed as a function of gamma-ray energy. The radioactivities of 234Th and 234mPa and 21.72 times that of 235U are equal to the radioactivity of 235U in natural uranium. Therefore, the plot of 21.72-fold R/B for 235U should be on a curve fitted to the points for 234Th and 234mPa in natural uranium. Depleted uranium with a 235U isotopic composition of less than 0.68% could be discriminated from natural uranium in the case of a reagent containing 4.0 g of uranium. PMID:11393763

  4. Semi-automated structural analysis of high resolution magnetic and gamma-ray spectrometry airborne surveys

    NASA Astrophysics Data System (ADS)

    Debeglia, N.; Martelet, G.; Perrin, J.; Truffert, C.; Ledru, P.; Tourlière, B.

    2005-08-01

    A user-controlled procedure was implemented for the structural analysis of geophysical maps. Local edge segments are first extracted using a suitable edge detector function, then linked into straight discontinuities and, finally, organised in complex boundary lines best delineating geophysical features. Final boundary lines may be attributed by a geologist to lithological contacts and/or structural geological features. Tests of some edge detectors, (i) horizontal gradient magnitude (HGM), (ii) various orders of the analytic signal ( An), reduced to the pole or not, (iii) enhanced horizontal derivative (EHD), (iv) composite analytic signal (CAS), were performed on synthetic magnetic data (with and without noise). As a result of these comparisons, the horizontal gradient appears to remain the best operator for the analysis of magnetic data. Computation of gradients in the frequency domain, including filtering and upward continuation of noisy data, is well-suited to the extraction of magnetic gradients associated to deep sources, while space-domain smoothing and differentiation techniques is generally preferable in the case of shallow magnetic sources, or for gamma-ray spectrometry analysis. Algorithms for edge extraction, segment linking, and line following can be controlled by choosing adequate edge detector and processing parameters which allows adaptation to a desired scale of interpretation. Tests on synthetic and real case data demonstrate the adaptability of the procedure and its ability to produce basic layer for multi-data analysis. The method was applied to the interpretation of high-resolution airborne magnetic and gamma-ray spectrometry data collected in northern Namibia. It allowed the delineation of dyke networks concealed by superficial weathering and demonstrated the presence of lithological variations in alluvial flows. The output from the structural analysis procedure are compatible with standard GIS softwares and enable the geologist to (i) compare

  5. The Study of Equilibrium factor between Radon-222 and its Daughters in Bangkok Atmosphere by Gamma-ray Spectrometry

    NASA Astrophysics Data System (ADS)

    Rujiwarodom, Rachanee

    2010-05-01

    To study the Equilibrium between radon-222 and its daughters in Bangkok atmosphere by Gamma-ray spectrometry, air sample were collected on 48 activated charcoal canister and 360 glass fiber filters by using a high volume jet-air sampler during December 2007 to November 2008.The Spectra of gamma-ray were measured by using a HPGe (Hyper Pure Germanium Detector). In the condition of secular equilibrium obtaining between Radon-222 and its decay products, radon-222 on activated charcoal canister and its daughters on glass fiber filters collected in the same time interval were calculated. The equilibrium factor (F) in the open air had a value of 0.38 at the minimum ,and 0.75 at the maximum. The average value of equilibrium factor (F) was 0.56±0.12. Based on the results, F had variations with a maximum value in the night to the early morning and decreased in the afternoon. In addition, F was higher in the winter than in the summer. This finding corresponds with the properties of the Earth atmosphere. The equilibrium factor (F) also depended on the concentration of dust in the atmosphere. People living in Bangkok were exposed to average value of 30 Bq/m3 of Radon-222 in the atmosphere. The equilibrium factor (0.56±0.12) and the average value of Radon-222 showed that people were exposed to alpha energy from radon-222 and its daughters decay at 0.005 WL(Working Level) which is lower than the safety standard at 0.02 WL. Keywords: Radon, Radon daughters , equilibrium factor, Gamma -ray spectrum analysis ,Bangkok ,Thailand

  6. Evaluation of Monte Carlo-based calibrations of HPGe detectors for in situ gamma-ray spectrometry.

    PubMed

    Boson, Jonas; Plamboeck, Agneta H; Ramebäck, Henrik; Agren, Göran; Johansson, Lennart

    2009-11-01

    The aim of this work was to evaluate the use of Monte Carlo-based calibrations for in situ gamma-ray spectrometry. We have performed in situ measurements at five different sites in Sweden using HPGe detectors to determine ground deposition activity levels of (137)Cs from the 1986 Chernobyl accident. Monte Carlo-calculated efficiency calibration factors were compared with corresponding values calculated using a more traditional semi-empirical method. In addition, results for the activity ground deposition were also compared with activity densities found in soil samples. In order to facilitate meaningful comparisons between the different types of results, the combined standard uncertainty of in situ measurements was assessed for both calibration methods. Good agreement, both between the two calibration methods, and between in situ measurements and soil samples, was found at all five sites. Uncertainties in in situ measurements for the given measurement conditions, about 20 years after the fallout occurred, were found to be in the range 15-20% (with a coverage factor k=1, i.e. with a confidence interval of about 68%). PMID:19604609

  7. A new measurement of the rare decay eta -> pi^0 gamma gamma with the Crystal Ball/TAPS detectors at the Mainz Microtron

    SciTech Connect

    Nefkens, B M; Prakhov, S; Aguar-Bartolom��, P; Annand, J R; Arends, H J; Bantawa, K; Beck, R; Bekrenev, V; Bergh��user, H; Braghieri, A; Briscoe, W J; Brudvik, J; Cherepnya, S; Codling, R F; Collicott, C; Costanza, S; Danilkin, I V; Denig, A; Demissie, B; Dieterle, M; Downie, E J; Drexler, P; Fil'kov, L V; Fix, A; Garni, S; Glazier, D I; Gregor, R; Hamilton, D; Heid, E; Hornidge, D; Howdle, D; Jahn, O; Jude, T C; Kashevarov, V L; K��ser, A; Keshelashvili, I; Kondratiev, R; Korolija, M; Kotulla, M; Koulbardis, A; Kruglov, S; Krusche, B; Lisin, V; Livingston, K; MacGregor, I J; Maghrbi, Y; Mancel, J; Manley, D M; McNicoll, E F; Mekterovic, D; Metag, V; Mushkarenkov, A; Nikolaev, A; Novotny, R; Oberle, M; Ortega, H; Ostrick, M; Ott, P; Otte, P B; Oussena, B; Pedroni, P; Polonski, A; Robinson, J; Rosner, G; Rostomyan, T; Schumann, S; Sikora, M H; Starostin, A; Strakovsky, I I; Strub, T; Suarez, I M; Supek, I; Tarbert, C M; Thiel, M; Thomas, A; Unverzagt, M; Watts, D P; Werthmueller, D; Witthauer, L

    2014-08-01

    A new measurement of the rare, doubly radiative decay eta->pi^0 gamma gamma was conducted with the Crystal Ball and TAPS multiphoton spectrometers together with the photon tagging facility at the Mainz Microtron MAMI. New data on the dependence of the partial decay width, Gamma(eta->pi^0 gamma gamma), on the two-photon invariant mass squared, m^2(gamma gamma), as well as a new, more precise value for the decay width, Gamma(eta->pi^0 gamma gamma) = (0.33+/-0.03_tot) eV, are based on analysis of 1.2 x 10^3 eta->pi^0 gamma gamma decays from a total of 6 x 10^7 eta mesons produced in the gamma p -> eta p reaction. The present results for dGamma(eta->pi^0 gamma gamma)/dm^2(gamma gamma) are in good agreement with previous measurements and recent theoretical calculations for this dependence.

  8. Experimental determination of the self-absorption factor for MTR plates by passive gamma spectrometric measurement

    NASA Astrophysics Data System (ADS)

    Berndt, R.; Mortreau, P.

    2011-07-01

    The measurement of the absolute activity or the mass of radioactive substances by gamma spectrometry needs to include a correction for the radiation absorption inside the source volume, the so-called self-absorption factor. It depends on geometry and material composition of the source, the detector geometry and on the geometrical arrangement of source and gamma radiation detector; it can be calculated if full information about all that is available. This article however describes how to determine the self-absorption factor from measurements if the radiation sources are plates of uranium fuel with typical parameters of nuclear fuel for MTR reactors and without using detail information on the source geometry, thus allowing easy inspection without relying on - potentially falsified - declarations on the internal properties of the fuel objects and without calculation.

  9. Gamma-ray spectrometry of granitic suites of the Paranaguá Terrane, Southern Brazil

    NASA Astrophysics Data System (ADS)

    Weihermann, Jessica Derkacz; Ferreira, Francisco José Fonseca; Cury, Leonardo Fadel; da Silveira, Claudinei Taborda

    2016-09-01

    The Paranaguá Terrane, located in the coastal portion of the states of Santa Catarina, Paraná and São Paulo in Southern Brazil is a crustal segment constituted mainly by an igneous complex, with a variety of granitic rocks inserted into the Serra do Mar ridge. The average altitude is approximately 1200 m above sea level, with peaks of up to 1800 m. Due to the difficulty of accessing the area, a shortage of outcrops and the thick weathering mantle, this terrane is understudied. This research aims to evaluate the gamma-ray spectrometry data of the granitic suites of the Paranaguá Terrane, in correspondence with the geological, petrographical, lithogeochemical, relief and mass movement information available in the literature. Aerogeophysical data were acquired along north-south lines spaced at 500 m, with a mean terrain clearance of 100 m. These data cover potassium (K, %), equivalent in thorium (eTh, ppm) and equivalent in uranium (eU, ppm). After performing a critical analysis of the data, basic (K, eU, eTh) and ternary (R-K/G-eTh/B-eU) maps were generated and then superimposed on the digital elevation model (DEM). The investigation of the radionuclide mobility across the relief and weathering mantle consisted of an analysis of the schematic profiles of elevation related with each radionuclide; a comparison of the K, eU and eTh maps with their 3D correspondents; and the study of mass movements registered in the region. A statistical comparison of lithogeochemical (K, U, Th) and geophysical (K, eU, eTh) data showed consistency in all the granitic suites studied (Morro Inglês, Rio do Poço and Canavieiras-Estrela). Through gamma-ray spectrometry, it was possible to establish relationships between scars (from mass movements) and the gamma-ray responses as well as the radionuclide mobility and the relief and to map the granitic bodies.

  10. Precision Measurement of {eta} --> {gamma} {gamma} Decay Width via the Primakoff Effect

    SciTech Connect

    Gan, Liping Gin

    2013-08-01

    A precision measurement of the {eta} --> {gamma} {gamma} decay width via the Primakoff effect is underway in Hall D at Jefferson Lab. The decay width will be extracted from measured differential cross sections at forward angles on two light targets, liquid hydrogen and 4He, using a 11.5 GeV tagged photon beam. Results of this experiment will not only potentially resolve a long standing discrepancy between the Primakoff and the collider measurements, but will also reduce the experimental uncertainty by a factor of two on the average value of previous experimental results listed by the Particle Data Group(PDG). It will directly improve all other eta partial decay widths which rely on the accuracy of the eta radiative decay width. The projected 3% precision on the {Gamma}({eta} --> {gamma} {gamma} ) measurement will have a significant impact on the experimental determination of the fundamental parameters in QCD, such as the ratio of light quark masses (m{sub u},m{sub d},m{sub s}) and the {eta} - {eta}' mixing angle. It will be a sensitive probe for understanding QCD symmetries and the origin and the dynamics of QCD symmetry breaking.

  11. Development and calibration of a real-time airborne radioactivity monitor using direct gamma-ray spectrometry with two scintillation detectors.

    PubMed

    Casanovas, R; Morant, J J; Salvadó, M

    2014-07-01

    The implementation of in-situ gamma-ray spectrometry in an automatic real-time environmental radiation surveillance network can help to identify and characterize abnormal radioactivity increases quickly. For this reason, a Real-time Airborne Radioactivity Monitor using direct gamma-ray spectrometry with two scintillation detectors (RARM-D2) was developed. The two scintillation detectors in the RARM-D2 are strategically shielded with Pb to permit the separate measurement of the airborne isotopes with respect to the deposited isotopes.In this paper, we describe the main aspects of the development and calibration of the RARM-D2 when using NaI(Tl) or LaBr3(Ce) detectors. The calibration of the monitor was performed experimentally with the exception of the efficiency curve, which was set using Monte Carlo (MC) simulations with the EGS5 code system. Prior to setting the efficiency curve, the effect of the radioactive source term size on the efficiency calculations was studied for the gamma-rays from (137)Cs. Finally, to study the measurement capabilities of the RARM-D2, the minimum detectable activity concentrations for (131)I and (137)Cs were calculated for typical spectra at different integration times. PMID:24607535

  12. Assay for uranium and determination of disequilibrium by means of in situ high resolution gamma-ray spectrometry

    USGS Publications Warehouse

    Tanner, Allan B.; Moxham, Robert M.; Senftle, F.E.

    1977-01-01

    Two sealed sondes, using germanium gamma-ray detectors cooled by melting propane, have been field tested to depths of 79 m in water-filled boreholes at the Pawnee Uranium Mine in Bee Co., Texas. When, used as total-count devices, the sondes are comparable in logging speed and counting rate with conventional scintillation detectors for locating zones of high radioactivity. When used with a multichannel analyzer, the sondes are detectors with such high resolution that individual lines from the complex spectra of the uranium and thorium series can be distinguished. Gamma rays from each group of the uranium series can be measured in ore zones permitting determination of the state of equilibrium at each measurement point. Series of 10-minute spectra taken at 0.3- to 0.5-m intervals in several holes showed zones where maxima from the uranium group and from the 222Rn group were displaced relative to each other. Apparent excesses of 230Th at some locations suggest that uranium-group concentrations at those locations were severalfold greater some tens of kiloyears, ago. At the current state of development a 10-minute count yields a sensitivity of about 80 ppm U308. Data reduction could in practice be accomplished in about 5 minutes. The result is practically unaffected by disequilibrium or radon contamination. In comparison with core assay, high-resolution spectrometry samples a larger volume; avoids problems due to incomplete core recovery, loss of friable material to drilling fluids, and errors in depth and marking; and permits use of less expensive drilling methods. Because gamma rays from the radionuclides are accumulated simultaneously, it also avoids the problems inherent in trying to correlate logs made in separate runs with different equipment. Continuous-motion delayed-gamma activation by a 163-?g 252Cf neutron source attached to the sonde yielded poor sensitivity. A better neutron-activation method, in which the sonde is moved in steps so as to place the detector

  13. Gamma densitometry for the measurement of skeletal density

    NASA Astrophysics Data System (ADS)

    Chalker, B. E.; Barnes, D. J.

    1990-03-01

    A method is described for the measurement of the density of calcium carbonate materials from the attenuation of a narrow, collimated beam of gamma photons. For the measurement of density for slices, approximately 0.5 to 1.0 cm thick, from the skeletons of reef building corals, the optimum beam energy is 30 34 keV; and measurement is practical from approximately 22 to 100 keV. The potential utilities of five commercially available isotopic sources (109Cd,125I,253Gd,210Pb and241Am) are evaluated. Methods and results are presented for gamma densitometry using210Pb and241Am. The210Pb point source had its principal gamma emission at 46.5 keV. Bremsstrahlung and high energy (800 keV) gamma emissions associated with the210Pb decay grand-daughter were detected, and procedures were developed to accommodate the contribution of these emissions to the overall count rate. The attenuation of count rate by aluminium and aragonite absorbers closely followed simple theoretical considerations provided that narrow energy window settings were used at the radiation monitor. These theoretical considerations take account of the density of the material absorbing the radiation, and hence the density could be determined from the attenuation of the gamma beam. Increased accuracy was achieved by the use of241Am and high speed counting equipment.241Am has its principal gamma emission at 59.6 keV. The attenuation of this gamma beam follows simple theoretical considerations for targets with mass thicknesses from 0 to 6 g cm-2. Aragonite from the shell of a giant clam was found to have slightly different properties in the absorption of gamma photons to aragonite from a coral skeleton. The differences were small but statistically significant.

  14. Measurement of ²²⁶Ra in soil from oil field: advantages of γ-ray spectrometry and application to the IAEA-448 CRM.

    PubMed

    Ceccatelli, A; Katona, R; Kis-Benedek, G; Pitois, A

    2014-05-01

    The analytical performance of gamma-ray spectrometry for the measurement of (226)Ra in TENORM (Technically Enhanced Naturally Occurring Radioactive Material) soil was investigated by the IAEA. Fast results were obtained for characterization and certification of a new TENORM Certified Reference Material (CRM), identified as IAEA-448 (soil from oil field). The combined standard uncertainty of the gamma-ray spectrometry results is of the order of 2-3% for massic activity measurement values ranging from 16500 Bq kg(-1) to 21500 Bq kg(-1). Methodologies used for the production and certification of the IAEA-448 CRM are presented. Analytical results were confirmed by alpha spectrometry. The "t" test showed agreement between alpha and gamma results at 95% confidence level.

  15. Radon loss from encapsulated sediments in Ge gamma-ray spectrometry for the annual radiation dose determination in luminescence dating

    NASA Astrophysics Data System (ADS)

    de Corte, F.; Vandenberghe, D.; de Wispelaere, A.; Buylaert, J.-P.; van den Haute, P.

    2006-01-01

    In Ge gamma-ray spectrometry for the annual radiation dose determination in the luminescence dating of sediments, the picture of 226Ra enrichment or depletion (in the 238U decay series) obtained via measurement of its 214Pb and 214Bi daughters may be disturbed by the 222Rn-content of the sample being decreased due to manipulations such as drying and pulverizing. Therefore, it is common practice to start the measurement only about 1 month after encapsulating the material, after which the 226Ra(1600 a)- 222Rn(3.82 d) mother-daughter equilibrium is re-established. Evidently, this only holds on condition that no significant escape of Rn occurs out of the sediment after making it up for counting. In order to experimentally investigate this effect, in the present work measurements were carried out with various types of dried and pulverized sediments that were either encapsulated in screw-cap polystyrene vials or in sealed glass containers, or that were mixed with molten wax followed by solidification in a cylindrical geometry. From the results obtained, it could be concluded that preparation and counting of the sediment-wax mixture is the method of choice.

  16. Recent gamma background measurements at high mountain altitude.

    PubMed

    Mishev, A L; Hristova, E

    2012-11-01

    Results from recent measurements of radiation gamma background at high mountain altitude, namely at Basic Environmental Observatory Moussala (42.11 N, 23.35 E, 2925 m a.s.l.) are reported. The measurements are fulfilled with several devices, namely IGS-421 gamma probe and MDU Liulin. A comparative analysis with previous measurements performed with SBN-90 SAPHYMO NaI(Tl) gamma probe is carried out. A temperature effect during winter period of SAPHYMO probe is observed. In addition the measurements are compared with CaSO(4):Dy TLD. The obtained results are widely discussed. A numerical model for galactic cosmic ray contribution to the dose rate in air is presented. The model is based on a full Monte Carlo simulation of cosmic ray induced cascade in the atmosphere. The simulation is carried out with CORSIKA 6.52 code using FLUKA 2006b and QGSJET II hadron interaction models. PMID:22659148

  17. Measurement of background gamma radiation in the northern Marshall Islands

    PubMed Central

    Bordner, Autumn S.; Crosswell, Danielle A.; Katz, Ainsley O.; Shah, Jill T.; Zhang, Catherine R.; Nikolic-Hughes, Ivana; Hughes, Emlyn W.; Ruderman, Malvin A.

    2016-01-01

    We report measurements of background gamma radiation levels on six islands in the northern Marshall Islands (Enewetak, Medren, and Runit onEnewetak Atoll; Bikini and Nam on Bikini Atoll; and Rongelap on Rongelap Atoll). Measurable excess radiation could be expected from the decay of 137Cs produced by the US nuclear testing program there from 1946 to 1958. These recordings are of relevance to safety of human habitation and resettlement. We find low levels of gamma radiation for the settled island of Enewetak [mean = 7.6 millirem/year (mrem/y) = 0.076 millisievert/year (mSv/y)], larger levels of gamma radiation for the island of Rongelap (mean = 19.8 mrem/y = 0.198 mSv/y), and relatively high gamma radiation on the island of Bikini (mean = 184 mrem/y = 1.84 mSv/y). Distributions of gamma radiation levels are provided, and hot spots are discussed. We provide interpolated maps for four islands (Enewetak, Medren, Bikini, and Rongelap), and make comparisons to control measurements performed on the island of Majuro in the southern Marshall Islands, measurements made in Central Park in New York City, and the standard agreed upon by the United States and the Republic of the Marshall Islands (RMI) governments (100 mrem/y = 1 mSv/y). External gamma radiation levels on Bikini Island significantly exceed this standard (P = <<0.01), and external gamma radiation levels on the other islands are below the standard. To determine conclusively whether these islands are safe for habitation, radiation exposure through additional pathways such as food ingestion must be considered. PMID:27274073

  18. Measurement of background gamma radiation in the northern Marshall Islands.

    PubMed

    Bordner, Autumn S; Crosswell, Danielle A; Katz, Ainsley O; Shah, Jill T; Zhang, Catherine R; Nikolic-Hughes, Ivana; Hughes, Emlyn W; Ruderman, Malvin A

    2016-06-21

    We report measurements of background gamma radiation levels on six islands in the northern Marshall Islands (Enewetak, Medren, and Runit onEnewetak Atoll; Bikini and Nam on Bikini Atoll; and Rongelap on Rongelap Atoll). Measurable excess radiation could be expected from the decay of (137)Cs produced by the US nuclear testing program there from 1946 to 1958. These recordings are of relevance to safety of human habitation and resettlement. We find low levels of gamma radiation for the settled island of Enewetak [mean = 7.6 millirem/year (mrem/y) = 0.076 millisievert/year (mSv/y)], larger levels of gamma radiation for the island of Rongelap (mean = 19.8 mrem/y = 0.198 mSv/y), and relatively high gamma radiation on the island of Bikini (mean = 184 mrem/y = 1.84 mSv/y). Distributions of gamma radiation levels are provided, and hot spots are discussed. We provide interpolated maps for four islands (Enewetak, Medren, Bikini, and Rongelap), and make comparisons to control measurements performed on the island of Majuro in the southern Marshall Islands, measurements made in Central Park in New York City, and the standard agreed upon by the United States and the Republic of the Marshall Islands (RMI) governments (100 mrem/y = 1 mSv/y). External gamma radiation levels on Bikini Island significantly exceed this standard (P = <0.01), and external gamma radiation levels on the other islands are below the standard. To determine conclusively whether these islands are safe for habitation, radiation exposure through additional pathways such as food ingestion must be considered.

  19. Measurement of background gamma radiation in the northern Marshall Islands.

    PubMed

    Bordner, Autumn S; Crosswell, Danielle A; Katz, Ainsley O; Shah, Jill T; Zhang, Catherine R; Nikolic-Hughes, Ivana; Hughes, Emlyn W; Ruderman, Malvin A

    2016-06-21

    We report measurements of background gamma radiation levels on six islands in the northern Marshall Islands (Enewetak, Medren, and Runit onEnewetak Atoll; Bikini and Nam on Bikini Atoll; and Rongelap on Rongelap Atoll). Measurable excess radiation could be expected from the decay of (137)Cs produced by the US nuclear testing program there from 1946 to 1958. These recordings are of relevance to safety of human habitation and resettlement. We find low levels of gamma radiation for the settled island of Enewetak [mean = 7.6 millirem/year (mrem/y) = 0.076 millisievert/year (mSv/y)], larger levels of gamma radiation for the island of Rongelap (mean = 19.8 mrem/y = 0.198 mSv/y), and relatively high gamma radiation on the island of Bikini (mean = 184 mrem/y = 1.84 mSv/y). Distributions of gamma radiation levels are provided, and hot spots are discussed. We provide interpolated maps for four islands (Enewetak, Medren, Bikini, and Rongelap), and make comparisons to control measurements performed on the island of Majuro in the southern Marshall Islands, measurements made in Central Park in New York City, and the standard agreed upon by the United States and the Republic of the Marshall Islands (RMI) governments (100 mrem/y = 1 mSv/y). External gamma radiation levels on Bikini Island significantly exceed this standard (P = <0.01), and external gamma radiation levels on the other islands are below the standard. To determine conclusively whether these islands are safe for habitation, radiation exposure through additional pathways such as food ingestion must be considered. PMID:27274073

  20. Lunar Elemental Abundances from Gamma-Ray and Neutron Measurements

    NASA Astrophysics Data System (ADS)

    Reedy, R. C.; Vaniman, D. T.

    1999-01-01

    The determination of elemental abundances is one of the highest science objectives of most lunar missions. Such multi-element abundances, ratios, or maps should include results for elements that are diagnostic or important in lunar processes, including heat-producing elements (such as K and Th), important incompatible elements (Th and rare earth elements), H (for polar deposits and regolith maturity), and key variable elements in major lunar provinces (such as Fe and Ti in the maria). Both neutron and gamma-ray spectroscopy can be used to infer elemental abundances; the two complement each other. These elemental abundances need to be determined with high accuracy and precision from measurements such as those made by the gamma-ray spectrometer (GRS) and neutron spectrometers (NS) on Lunar Prospector. As presented here, a series of steps, computer codes, and nuclear databases are needed to properly convert the raw gamma-ray and neutron measurements into good elemental abundances, ratios, and/or maps. Lunar Prospector (LP) is the first planetary mission that has measured neutrons escaping from a planet other than the Earth. The neutron spectrometers on Lunar Prospector measured a wide range of neutron energies. The ability to measure neutrons with thermal (E < 0.1 eV), epithermal (E about equal 0.1 - 1000 eV), and fast (E about 0.1-10 MeV) energies maximizes the scientific return, being especially sensitive to both H (using epithermal neutrons) and thermal-neutron-absorbing elements. Neutrons are made in the lunar surface by the interaction of galactic-cosmic-ray (GCR) particles with the atomic nuclei in the surface. Most neutrons are produced with energies above about 0.1 MeV. The flux of fast neutrons in and escaping from the Moon depends on es the intensity of the cosmic rays (which vary with solar activity) and the elemental composition of the surface. Variations in the elemental composition of the lunar surface can affect the flux of fast neutrons by about 25

  1. Gamma densitometer for measuring Pu density in fuel tubes

    SciTech Connect

    Winn, W.G.

    1982-01-01

    A fuel-gamma-densitometer (FGD) has been developed to examine nondestructively the uniformity of plutonium in aluminum-clad fuel tubes at the Savannah River Plant (SRP). The monitoring technique is ..gamma..-ray spectroscopy with a lead-collimated Ge(Li) detector. Plutonium density is correlated with the measured intensity of the 208 keV ..gamma..-ray from /sup 237/U (7d) of the /sup 241/Pu (15y) decay chain. The FGD measures the plutonium density within 0.125- or 0.25-inch-diameter areas of the 0.133- to 0.183-inch-thick tube walls. Each measurement yields a density ratio that relates the plutonium density of the measured area to the plutonium density in normal regions of the tube. The technique was used to appraise a series of fuel tubes to be irradated in an SRP reactor. High-density plutonium areas were initially identified by x-ray methods and then examined quantitatively with the FGD. The FGD reliably tested fuel tubes and yielded density ratios over a range of 0.0 to 2.5. FGD measurements examined (1) nonuniform plutonium densities or hot spots, (2) uniform high-density patches, and (3) plutonium density distribution in thin cladding regions. Measurements for tubes with known plutonium density agreed with predictions to within 2%. Attenuation measurements of the 208-keV ..gamma..-ray passage through the tube walls agreed to within 2 to 3% of calculated predictions. Collimator leakage measurements agreed with model calculations that predicted less than a 1.5% effect on plutonium density ratios. Finally, FGD measurements correlated well with x-ray transmission and fluoroscopic measurements. The data analysis for density ratios involved a small correction of about 10% for ..gamma..-shielding within the fuel tube. For hot spot examinations, limited information for this correction dictated a density ratio uncertainty of 3 to 5%.

  2. Practical applicability of field gamma-ray scintillation spectrometry in geophysical surveys

    PubMed

    Chiozzi; Pasquale; Verdoya; De Felice P

    2000-07-01

    We discuss the problems and calibration procedures for a portable gamma-ray scintillation spectrometer for determinations of potassium, uranium and thorium concentration in rocks. Particular emphasis was given to the evaluation of the background radiation. The apparatus was tested in the field at two selected areas in NW Italy. We found appropriate sites which could be used as reference targets to frequently check the gamma-ray equipment. An area formed by serpentinitic rocks showed such a low measured radioactivity that it could be used as a reference for the local background effect. An anomalously high uranium amount against negligible potassium and thorium concentrations were found in outcrops of dolomitic rocks, which can be used to detect possible changes in the instrument calibration constants.

  3. A COMPARISON OF GADRAS SIMULATED AND MEASURED GAMMA RAY SPECTRA

    SciTech Connect

    Jeffcoat, R.; Salaymeh, S.

    2010-06-28

    Gamma-ray radiation detection systems are continuously being developed and improved for detecting the presence of radioactive material and for identifying isotopes present. Gamma-ray spectra, from many different isotopes and in different types and thicknesses of attenuation material and matrixes, are needed to evaluate the performance of these devices. Recently, a test and evaluation exercise was performed by the Savannah River National Laboratory that required a large number of gamma-ray spectra. Simulated spectra were used for a major portion of the testing in order to provide a pool of data large enough for the results to be statistically significant. The test data set was comprised of two types of data, measured and simulated. The measured data were acquired with a hand-held Radioisotope Identification Device (RIID) and simulated spectra were created using Gamma Detector Response and Analysis Software (GADRAS, Mitchell and Mattingly, Sandia National Laboratory). GADRAS uses a one-dimensional discrete ordinate calculation to simulate gamma-ray spectra. The measured and simulated spectra have been analyzed and compared. This paper will discuss the results of the comparison and offer explanations for spectral differences.

  4. Gamma-ray spectrometry across the Aalenian-Bajocian boundary in the Lusitanian Basin (Western Portugal)

    NASA Astrophysics Data System (ADS)

    Santos, Marisa; Henriques, Helena; Pena, Rui

    2016-04-01

    supply, which has enabled the faunal recovery, as well as the raise of deep infaunal foraminifers recorded at the latest part of the Discites Biochron. This could be related to the increase of calcareous nannofossil fluxes that coincide with a positive shift in carbon isotope compositions of bulk carbonate in the earliest Bajocian reported by some authors for the Murtinheira and other Iberian sections. In basin analysis of carbonate platforms the integration of major biotic turnovers and gamma-ray spectrometry data can be a useful tool in the improvement of correlation between wells and outcrops. Moreover, they assist in the interpretation of depositional environment and paleoclimatic constrains assigned to a basin.

  5. Systematic Effects on Duration Measurements of Gamma-Ray Bursts

    NASA Technical Reports Server (NTRS)

    Koshut, Thomas M.; Paciesas, William S.; Kouveliotou, Chryssa; vanParadijs, Jan; Pendleton, Geoffrey N.; Fishman, Gerald J.; Meegan, Charles A.

    1996-01-01

    The parameters T(sub 90) and T(sub 50) have recently been introduced as a measurement of the duration of gamma-ray bursts. We present here a description of the method of measuring T(sub 90) and T(sub 50) and its application to gamma-ray bursts observed with the Burst and Transient Source Experiment (BATSE) onboard the Compton Gamma-Ray Observatory (CGRO). We use simulated as well as observed time profiles to address some of the possible systematic effects affecting individual T(sub 90) (T(sub 50)) measurements. We show that these systematic effects do not mimic those effects that would result from time dilation if the burst sources are at distances of several Gpc. We discuss the impact of these systematic effects on the T(sub 90) (T(sub 50)) distributions for the gamma-ray bursts observed with BATSE. We distinguish between various types of T(sub 90) (T(sub 50)) distributions, and discuss the ways in which distributions observed with different experiments can vary, even though the measurements for commonly observed bursts may be the same. We then discuss the distributions observed with BATSE and compare them to those observed with other experiments.

  6. Determination of 137Cs activity in soil from Qatar using high-resolution gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Al-Sulaiti, Huda; Nasir, Tabassum; Al Mugren, K. S.; Alkhomashi, N.; Al-Dahan, N.; Al-Dosari, M.; Bradley, D. A.; Bukhari, S.; Matthews, M.; Regan, P. H.; Santawamaitre, T.; Malain, D.; Habib, A.; Al-Dosari, Hanan; Al Sadig, Ibrahim; Daar, Eman

    2016-10-01

    With interest in establishing baseline concentrations of 137Cs in soil from the Qatarian peninsula, we focus on determination of the activity concentrations in 129 soil samples collected across the State of Qatar prior to the 2011 Fukushima Dai-ichi nuclear power plant accident. As such, the data provides the basis of a reference map for the detection of releases of this fission product. The activity concentrations were measured via high-resolution gamma-ray spectrometry using a hyper-pure germanium detector enclosed in a copper-lined passive lead shield that was situated in a low-background environment. The activity concentrations ranged from 0.21 to 15.41 Bq/kg, with a median value of 1 Bq/kg, the greatest activity concentration being observed in a sample obtained from northern Qatar. Although it cannot be confirmed, it is expected that this contamination is mainly due to releases from the Chernobyl accident of 26 April 1986, there being a lack of data from Qatar before the accident. The values are typically within but are sometimes lower than the range indicated by data from other countries in the region. The lower values than those of others is suggested to be due to variation in soil characteristics as well as metrological factors at the time of deposition.

  7. Resonance Ionization Mass Spectrometry System for Measurement of Environmental Samples

    NASA Astrophysics Data System (ADS)

    Pibida, L.; McMahon, C. A.; Nörtershäuser, W.; Bushaw, B. A.

    2002-10-01

    A resonance ionization mass spectrometry (RIMS) system has been developed at the National Institute of Standards and Technology (NIST) for sensitive and selective determination of radio-cesium in the environment. The overall efficiency was determined to be 4×10-7 with a combined (laser and mass spectrometer) selectivity of 108 for both 135Cs and 137Cs with respect to 133Cs. RIMS isotopic ratio measurements of 135Cs/ 137Cs were performed on a nuclear fuel burn-up sample and compared to measurements on a similar system at Pacific Northwest National Laboratory (PNNL) and to conventional thermal ionization mass spectrometry (TIMS). Results of preliminary RIMS investigations on a freshwater lake sediment sample are also discussed.

  8. Measurements of B to V(Gamma) Decays

    SciTech Connect

    Yarritu, Aaron K.; /Stanford U., Phys. Dept.

    2010-09-02

    The standard model has been highly successful at describing current experimental data. However, extensions of the standard model predict particles that have masses at energy scales that are above the electroweak scale. The flavor-changing neutral current processes of the B meson are sensitive to the influences of these new physics contributions. These processes proceed through loop diagrams, thus allowing new physics to enter at the same order as the standard model. New physics may contribute to the enhancement or suppression of rate asymmetries or the decay rates of these processes. The transition B {yields} V{gamma} (V = K*(892), {rho}(770), {omega}(782), {phi}(1020)) represents radiative decays of the B meson that proceed through penguin processes. Hadronic uncertainties limit the theoretical accuracy of the prediction of the branching fractions. However, uncertainties, both theoretical and experimental, are much reduced when considering quantities involving ratios of branching fractions, such as CP or isospin asymmetries. The most dominant exclusive radiative b {yields} s transition is B {yields} K*{gamma}. We present the best measurements of the branching fractions, direct CP, and isospin asymmetries of B {yields} K*{gamma}. The analogous b {yields} d transitions are B {yields} {rho}{gamma} and B {yields} {omega}{gamma}, which are suppressed by a factor of |V{sub td}/V{sub ts}|{sup 2} {approx} 0.04 relative to B {yields} K*{gamma}. A measurement of the branching fractions and isospin asymmetry of B{sup +} {yields} {rho}{sup +}{gamma} and B{sup 0} {yields} {rho}{sup 0}{gamma}, as well as a search for B {yields} {omega}{gamma}, are also given. These measurements are combined to calculate the ratio of CKM matrix elements |V{sub td}/V{sub ts}|, which corresponds to the length of one side of the unitary triangle. Finally, we present a search for the penguin annihilation process B {yields}{phi}{gamma}. We use a sample of 383 million B{bar B} events collected with

  9. Plutonium measurements by accelerator mass spectrometry at LLNL

    SciTech Connect

    McAninch, J E; Hamilton, T F; Broan, T A; Jokela, T A; Knezovich, T J; Ognibene, T J; Proctor, I D; Roberts, M L; Southon, J R; Vogel, J S; Sideras-Haddad, E

    1999-10-26

    Mass spectrometric methods provide sensitive, routine, and cost-effective analyses of long-lived radionuclides. Here the authors report on the status of work at Lawrence Livermore National Laboratory (LLNL) to develop a capability for actinide measurements by accelerator mass spectrometry (AMS) to take advantage of the high potential of AMS for rejection of interferences. This work demonstrates that the LLNL AMS spectrometer is well-suited for providing high sensitivity, robust, high throughput measurements of plutonium concentrations and isotope ratios. Present backgrounds are {approximately}2 x 10{sup 7}atoms per sample for environmental samples prepared using standard alpha spectrometry protocols. Recent measurements of {sup 239+240}Pu and {sup 241}Pu activities and {sup 240}Pu/{sup 239}Pu isotope ratios in IAEA reference materials agree well with IAEA reference values and with alpha spectrometry and recently published ICP-MS results. Ongoing upgrades of the AMS spectrometer are expected to reduce backgrounds below 1 x 10{sup 6} atoms per sample while allowing simplifications of the sample preparation chemistry. These simplifications will lead to lower per-sample costs, higher throughput, faster turn around and, ultimately, to larger and more robust data sets.

  10. Gamma Ray Mirrors for Direct Measurement of Spent Nuclear Fuel

    SciTech Connect

    Pivovaroff, Dr. Michael J.; Ziock, Klaus-Peter; Harrison, Mark J; Soufli, Regina

    2014-01-01

    Direct measurement of the amount of Pu and U in spent nuclear fuel represents a challenge for the safeguards community. Ideally, the characteristic gamma-ray emission lines from different isotopes provide an observable suitable for this task. However, these lines are generally lost in the fierce flux of radiation emitted by the fuel. The rates are so high that detector dead times limit measurements to only very small solid angles of the fuel. Only through the use of carefully designed view ports and long dwell times are such measurements possible. Recent advances in multilayer grazing-incidence gamma-ray optics provide one possible means of overcoming this difficulty. With a proper optical and coating design, such optics can serve as a notch filter, passing only narrow regions of the overall spectrum to a fully shielded detector that does not view the spent fuel directly. We report on the design of a mirror system and a number of experimental measurements.

  11. Measurement of the gamma gamma* to eta_c transition form factor

    SciTech Connect

    Lees, J.P.; Poireau, V.; Prencipe, E.; Tisserand, V.; Garra Tico, J.; Grauges, E.; Martinelli, M.; Palano, A.; Pappagallo, M.; Eigen, G.; Stugu, B.; Sun, L.; Battaglia, M.; Brown, D.N.; Hooberman, B.; Kerth, L.T.; Kolomensky, Yu.G.; Lynch, G.; Osipenkov, I.L.; Tanabe, T.; Hawkes, C.M.; /Birmingham U. /Ruhr U., Bochum /British Columbia U. /Brunel U. /Novosibirsk, IYF /UC, Irvine /UC, Riverside /UC, San Diego /UC, Santa Barbara /UC, Santa Cruz /Caltech /Cincinnati U. /Colorado U. /Colorado State U. /Dortmund U. /Dresden, Tech. U. /Ecole Polytechnique /Edinburgh U. /INFN, Ferrara /Ferrara U. /INFN, Ferrara /INFN, Ferrara /Ferrara U. /INFN, Ferrara /INFN, Ferrara /Ferrara U. /Frascati /INFN, Genoa /Genoa U. /INFN, Genoa /INFN, Genoa /Genoa U. /INFN, Genoa /INFN, Genoa /Genoa U. /Indian Inst. Tech., Guwahati /Harvard U. /Heidelberg U. /Humboldt U., Berlin /Imperial Coll., London /Iowa State U. /Iowa State U. /Johns Hopkins U. /Orsay, LAL /LLNL, Livermore /Liverpool U. /Queen Mary, U. of London /Royal Holloway, U. of London /Louisville U. /Mainz U., Inst. Kernphys. /Manchester U. /Maryland U. /Massachusetts U., Amherst /MIT /McGill U. /INFN, Milan /Milan U. /INFN, Milan /INFN, Milan /Milan U. /Mississippi U. /Montreal U. /INFN, Naples /Naples U. /NIKHEF, Amsterdam /NIKHEF, Amsterdam /Notre Dame U. /Ohio State U. /Oregon U. /INFN, Padua /Padua U. /INFN, Padua /INFN, Padua /Padua U. /Paris U., VI-VII /INFN, Perugia /Perugia U. /INFN, Pisa /Pisa U. /INFN, Pisa /Pisa, Scuola Normale Superiore /INFN, Pisa /Pisa U. /INFN, Pisa /Princeton U. /INFN, Rome /INFN, Rome /Rome U. /INFN, Rome /INFN, Rome /Rome U. /INFN, Rome /INFN, Rome /Rome U. /INFN, Rome /INFN, Rome /Rome U. /Rostock U. /Rutherford /DAPNIA, Saclay /SLAC /South Carolina U. /Stanford U., Phys. Dept. /SUNY, Albany /Tel Aviv U. /Tennessee U. /Texas Nuclear Corp., Austin /Texas U., Dallas /INFN, Turin /Turin U. /INFN, Trieste /Trieste U. /Valencia U. /Victoria U. /Warwick U. /Wisconsin U., Madison

    2010-04-28

    The authors study the reaction e{sup +}e{sup -} {yields} e{sup +}e{sup -} {eta}{sub c}, {eta}{sub c} {yields} K{sub S}K{sup {+-}}{pi}{sup {-+}} and obtain {eta}{sub c} mass and width values 2982.2 {+-} 0.4 {+-} 1.6 MeV/c{sup 2} and 31.7 {+-} 1.2 {+-} 0.8 MeV, respectively. They find {Lambda}({eta}{sub c} {yields} {gamma}{gamma}){Beta}({eta}{sub c} {yields} K{bar K}{pi}) = 0.374 {+-} 0.009 {+-} 0.031 keV, and measure the {gamma}{gamma}* {yields} {eta}{sub c} transition form factor in the momentum transfer range from 2 to 50 GeV{sup 2}. The analysis is based on 469 fb{sup -1} of integrated luminosity collected at PEP-II with the BABAR detector at e{sup +}e{sup -} center-of-mass energies near 10.6 GeV.

  12. Environmental gamma radiation measurement in district Swat, Pakistan.

    PubMed

    Jabbar, T; Khan, K; Subhani, M S; Akhter, P; Jabbar, A

    2008-01-01

    External exposure to environmental gamma ray sources is an important component of exposure to the public. A survey was carried out to determine activity concentration levels and associated doses from (226)Ra, (232)Th, (40)K and (137)Cs by means of high-resolution gamma ray spectrometry in the Swat district, famous for tourism. The mean concentrations for (226)Ra, (232)Th and (40)K were found to be 50.4 +/- 0.7, 34.8 +/- 0.7 and 434.5 +/- 7.4 Bq kg(-1), respectively, in soil samples, which are slightly more than the world average values. However, (137)Cs was only found in the soil sample of Barikot with an activity concentration of 34 +/- 1.2 Bq kg(-1). Only (40)K was determined in vegetation samples with an average activity of 172.2 +/- 1.7 Bq kg(-1), whereas in water samples, all radionuclides were found below lower limits of detection. The radium equivalent activity in all soil samples is lower than the limit set in the Organisation for Economic Cooperation and Development report (370 Bq kg(-1)). The value of the external exposure dose has been determined from the content of these radionuclides in soil. The average terrestrial gamma air absorbed dose rate was observed to be 62.4 nGy h(-1), which yields an annual effective dose of 0.08 mSv. The average value of the annual effective dose lies close to the global range of outdoor radiation exposure given in United Nations Scientific Committee on the Effects of Atomic Radiation. However, the main component of the radiation dose to the population residing in the study area arises from cosmic ray due to high altitude. PMID:18936087

  13. Neanderthal skeleton from Tabun: U-series data by gamma-ray spectrometry.

    PubMed

    Schwarcz, H P; Simpson, J J; Stringer, C B

    1998-12-01

    The Neanderthal hominid Tabun C1, found in Israel by Garrod & Bate, was attributed to either layer B or C of their stratigraphic sequence. We have used gamma-ray spectrometry to determine the 230Th/234U and 231Pa/235U ratios of two bones from this skeleton, the mandible and a femur. The ages calculated from these ratios depend on the uranium uptake history of the bones. Assuming a model of early U (EU) uptake the age of the Tabun C1 mandible is 34+/-5 ka. The EU age of the femur is 19+/-2 ka. The femur may have experienced continuous (linear) U uptake which would give an age of 33+/-4 ka, in agreement with the mandible's EU age, but implies marked inhomogeneity in U uptake history at the site. These new age estimates for the skeleton suggest that it was younger than deposits of layer C. This apparent age is less than those of other Neanderthals found in Israel, and distinctly younger than the ages of the Skhul and Qafzeh burials. This suggests that Neanderthals did not necessarily coexist with the earliest modern humans in the region. All of the more complete Neanderthal fossils from Israel are now dated to the cool period of the last glacial cycle, suggesting that Neanderthals may have arrived in this region as a result of the southward expansion of their habitable range. The young age determined for the Tabun skeleton would suggest that Neanderthals survived as late in the Levant as they did in Europe.

  14. Neanderthal skeleton from Tabun: U-series data by gamma-ray spectrometry.

    PubMed

    Schwarcz, H P; Simpson, J J; Stringer, C B

    1998-12-01

    The Neanderthal hominid Tabun C1, found in Israel by Garrod & Bate, was attributed to either layer B or C of their stratigraphic sequence. We have used gamma-ray spectrometry to determine the 230Th/234U and 231Pa/235U ratios of two bones from this skeleton, the mandible and a femur. The ages calculated from these ratios depend on the uranium uptake history of the bones. Assuming a model of early U (EU) uptake the age of the Tabun C1 mandible is 34+/-5 ka. The EU age of the femur is 19+/-2 ka. The femur may have experienced continuous (linear) U uptake which would give an age of 33+/-4 ka, in agreement with the mandible's EU age, but implies marked inhomogeneity in U uptake history at the site. These new age estimates for the skeleton suggest that it was younger than deposits of layer C. This apparent age is less than those of other Neanderthals found in Israel, and distinctly younger than the ages of the Skhul and Qafzeh burials. This suggests that Neanderthals did not necessarily coexist with the earliest modern humans in the region. All of the more complete Neanderthal fossils from Israel are now dated to the cool period of the last glacial cycle, suggesting that Neanderthals may have arrived in this region as a result of the southward expansion of their habitable range. The young age determined for the Tabun skeleton would suggest that Neanderthals survived as late in the Levant as they did in Europe. PMID:9929173

  15. Twin Knudsen Cell Configuration for Activity Measurements by Mass Spectrometry

    NASA Technical Reports Server (NTRS)

    Jacobson, N. S.

    1996-01-01

    A twin Knudsen cell apparatus for alloy activity measurements by mass spectrometry is described. Two Knudsen cells - one containing an alloy and one containing a pure component - are mounted on a single flange and translated into the sampling region via a motorized x-y table. Mixing of the molecular beams from the cells is minimized by a novel system of shutters. Activity measurements were taken on two well-characterized alloys to verify the operation of the system. Silver activity measurements are reported for Ag-Cu alloys and aluminum activity measurements are reported for Fe-Al alloys. The temperature dependence of activity for a 0.474 mol fraction Al-Fe alloy gives a partial molar heat of aluminum. Measurements taken with the twin cell show good agreement with literature values for these alloys.

  16. Implications of final L3 measurement of {sigma}{sub tot}({gamma}{gamma}{yields}bb)

    SciTech Connect

    Chyla, Jiri

    2006-02-01

    The excess of data on the total cross section of bb production in {gamma}{gamma} collisions over QCD predictions, observed by L3, OPAL and DELPHI Collaborations at LEP2, has so far defied explanation. The recent final analysis of L3 data has brought important new information concerning the dependence of the observed excess on the {gamma}{gamma} collisions energy W{sub {gamma}}{sub {gamma}}. The implications of this dependence are discussed.

  17. PWR and BWR spent fuel assembly gamma spectra measurements

    NASA Astrophysics Data System (ADS)

    Vaccaro, S.; Tobin, S. J.; Favalli, A.; Grogan, B.; Jansson, P.; Liljenfeldt, H.; Mozin, V.; Hu, J.; Schwalbach, P.; Sjöland, A.; Trellue, H.; Vo, D.

    2016-10-01

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative-Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. To compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.

  18. PWR and BWR spent fuel assembly gamma spectra measurements

    DOE PAGES

    Vaccaro, S.; Tobin, Stephen J.; Favalli, Andrea; Grogan, Brandon R.; Jansson, Peter; Liljenfeldt, Henrik; Mozin, Vladimir; Hu, Jianwei; Schwalbach, P.; Sjoland, A.; et al

    2016-07-17

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative–Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detectmore » the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. As a result, to compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.« less

  19. Airborne gamma radiation soil moisture measurements over short flight lines

    NASA Technical Reports Server (NTRS)

    Peck, Eugene L.; Carrol, Thomas R.; Lipinski, Daniel M.

    1990-01-01

    Results are presented on airborne gamma radiation measurements of soil moisture condition, carried out along short flight lines as part of the First International Satellite Land Surface Climatology Project Field Experiment (FIFE). Data were collected over an area in Kansas during the summers of 1987 and 1989. The airborne surveys, together with ground measurements, provide the most comprehensive set of airborne and ground truth data available in the U.S. for calibrating and evaluating airborne gamma flight lines. Analysis showed that, using standard National Weather Service weights for the K, Tl, and Gc radiation windows, the airborne soil moisture estimates for the FIFE lines had a root mean square error of no greater than 3.0 percent soil moisture. The soil moisture estimates for sections having acquisition time of at least 15 sec were found to be reliable.

  20. Accelerator mass spectrometry for measurement of long-lived radioisotopes.

    PubMed

    Elmore, D; Phillips, F M

    1987-05-01

    Particle accelerators, such as those built for research in nuclear physics, can also be used together with magnetic and electrostatic mass analyzers to measure rare isotopes at very low abundance ratios. All molecular ions can be eliminated when accelerated to energies of millions of electron volts. Some atomic isobars can be eliminated with the use of negative ions; others can be separated at high energies by measuring their rate of energy loss in a detector. The long-lived radioisotopes (10)Be, (14)C,(26)A1, 36Cl, and (129)1 can now be measured in small natural samples having isotopic abundances in the range 10(-12) to 10(- 5) and as few as 10(5) atoms. In the past few years, research applications of accelerator mass spectrometry have been concentrated in the earth sciences (climatology, cosmochemistry, environmental chemistry, geochronology, glaciology, hydrology, igneous petrogenesis, minerals exploration, sedimentology, and volcanology), in anthropology and archeology (radiocarbon dating), and in physics (searches for exotic particles and measurement of halflives). In addition, accelerator mass spectrometry may become an important tool for the materials and biological sciences. PMID:17740475

  1. Accelerator mass spectrometry for measurement of long-lived radioisotopes.

    PubMed

    Elmore, D; Phillips, F M

    1987-05-01

    Particle accelerators, such as those built for research in nuclear physics, can also be used together with magnetic and electrostatic mass analyzers to measure rare isotopes at very low abundance ratios. All molecular ions can be eliminated when accelerated to energies of millions of electron volts. Some atomic isobars can be eliminated with the use of negative ions; others can be separated at high energies by measuring their rate of energy loss in a detector. The long-lived radioisotopes (10)Be, (14)C,(26)A1, 36Cl, and (129)1 can now be measured in small natural samples having isotopic abundances in the range 10(-12) to 10(- 5) and as few as 10(5) atoms. In the past few years, research applications of accelerator mass spectrometry have been concentrated in the earth sciences (climatology, cosmochemistry, environmental chemistry, geochronology, glaciology, hydrology, igneous petrogenesis, minerals exploration, sedimentology, and volcanology), in anthropology and archeology (radiocarbon dating), and in physics (searches for exotic particles and measurement of halflives). In addition, accelerator mass spectrometry may become an important tool for the materials and biological sciences.

  2. Measurements of the CKM Angle phi3/gamma

    SciTech Connect

    Tisserand, Vincent; /Annecy, LAPP

    2007-06-27

    We present a review on the measurements of the CKM angle {gamma} ({phi}{sub 3}){sup 1} as performed by the BABAR and Belle experiments at the asymmetric-energy e{sup +}e{sup -} B factories colliders PEP-II and KEKB. These measurements are using either charged or neutral B decays. For charged B decays the modes {tilde D}{sup 0}K{sup -}, {tilde D}*{sup 0}K{sup -}, and {tilde D}{sup 0}K*{sup -} are employed, where {tilde D}{sup 0} indicates either a D{sup 0} or a {bar D}{sup 0} meson. Direct CP violation is exploited. It is caused by interferences between V{sub ub} and V{sub cb} accessible transitions that generate asymmetries in the final states. For these decays various methods exist to enhance the sensitivity to the V{sub ub} transition, carrying the weak phase {gamma}. For neutral B decays, the modes D{sup (*){+-}}{pi}{sup {-+}} and D{sup {+-}}{rho}{sup {-+}} are used. In addition to the V{sub ub} and V{sub cb} interferences, these modes are sensitive to the B{sup 0}-{bar B}{sup 0} mixing, so that time dependent analyses are performed to extract sin(2{beta} + {gamma}). An alternative method would use the lower branching ratios decay modes {tilde D}{sup (*)0}{bar K}{sup (*)0} where much larger asymmetries are expected. The various available methods are mostly ''theoretically clean'' and always free of penguins diagrams. In some cases a high sensitivity to {gamma} is expected and large asymmetries may be seen. But these measurements are always experimentally difficult as one has to face with either low branching ratios, or small asymmetries, or additional technical/theoretical difficulties due to Dalitz/SU(3) and re-scattering models needed to treat/estimate nuisance parameters such as unknown strong phases and the relative magnitude of the amplitude of the interfering ''V{sub ub}'' transitions. Thus at the present time only a relatively limited precision on {gamma} can be extracted from these measurements. The current world average is {gamma} = (78{sub -26}{sup +19

  3. Measurement of cross sections for the 63Cu(alpha,gamma)67Ga reaction from 5.9-8.7 MeV

    SciTech Connect

    Basunia, M. Shamsuzzoha; Norman, Eric B.; Shugart, Howard A.; Smith, Alan R.; Dolinski, Michelle J.; Quiter, Brian J.

    2004-09-23

    We have measured cross sections for the 63Cu(alpha,gamma)67Ga reaction in the 5.9-8.7 MeV energy range using an activation technique. Natural Cu foils were bombarded with alpha beams from the 88 Cyclotron at Lawrence Berkeley National Laboratory (LBNL). Activated foils were counted using gamma spectrometry system at LBNL's Low Background Facility. The 63Cu(alpha,gamma)67Ga cross-sections were determined and compared with the latest NON-SMOKER theoretical values. Experimental cross sections were found to be in agreement with theoretical values.

  4. PRESAGE 3D dosimetry accurately measures Gamma Knife output factors

    NASA Astrophysics Data System (ADS)

    Klawikowski, Slade J.; Yang, James N.; Adamovics, John; Ibbott, Geoffrey S.

    2014-12-01

    Small-field output factor measurements are traditionally very difficult because of steep dose gradients, loss of lateral electronic equilibrium, and dose volume averaging in finitely sized detectors. Three-dimensional (3D) dosimetry is ideal for measuring small output factors and avoids many of these potential challenges of point and 2D detectors. PRESAGE 3D polymer dosimeters were used to measure the output factors for the 4 mm and 8 mm collimators of the Leksell Perfexion Gamma Knife radiosurgery treatment system. Discrepancies between the planned and measured distance between shot centers were also investigated. A Gamma Knife head frame was mounted onto an anthropomorphic head phantom. Special inserts were machined to hold 60 mm diameter, 70 mm tall cylindrical PRESAGE dosimeters. The phantom was irradiated with one 16 mm shot and either one 4 mm or one 8 mm shot, to a prescribed dose of either 3 Gy or 4 Gy to the 50% isodose line. The two shots were spaced between 30 mm and 60 mm apart and aligned along the central axis of the cylinder. The Presage dosimeters were measured using the DMOS-RPC optical CT scanning system. Five independent 4 mm output factor measurements fell within 2% of the manufacturer’s Monte Carlo simulation-derived nominal value, as did two independent 8 mm output factor measurements. The measured distances between shot centers varied by ±0.8 mm with respect to the planned shot displacements. On the basis of these results, we conclude that PRESAGE dosimetry is excellently suited to quantify the difficult-to-measure Gamma Knife output factors.

  5. Neutron and Gamma Ray Scattering Measurements for Subsurface Geochemistry

    NASA Astrophysics Data System (ADS)

    Ellis, Darwin V.

    1990-10-01

    Developed for the oil industry, well logging instrumentation based on electrical, acoustic, and nuclear measurements has been providing information about the localization and evaluation of hydrocarbon-bearing strata for petroleum geologists and engineers since 1927. This method of exploring properties of the earth's crust without taking physical samples is attracting a growing audience of geologists and geophysicists because of recent developments that permit nondestructive measurements of subsurface geochemistry. A combination of nuclear measurement techniques, which use gamma ray and neutron sources, can provide detailed information on rock composition of interest to both industry and academia.

  6. Optimized background reduction in low-level gamma-ray spectrometry at a surface laboratory.

    PubMed

    Hurtado, S; García-León, M; García-Tenorio, R

    2006-09-01

    The background of a coaxial Ge detector placed at a surface laboratory has been reduced by means of a background reduction setup consisting of a passive shield of low-activity lead, a simple radon suppression system and an active shield with a plastic scintillation plate. In particular, we have devoted our efforts to in-depth optimization of each parameter associated with different anticoincidence setups and to their subsequent intercomparison. The overall performance of the active shield was improved by using the optimum time parameters for each setup. The final objective is to decrease the cosmic-ray background and, by this way, to reduce the detection limits of gamma-ray spectrometers at conventional laboratories, and consequently make them competitive for different measurements like (210)Pb dating.

  7. Fission Yield Measurements by Inductively Coupled Plasma Mass-Spectrometry

    SciTech Connect

    Irina Glagolenko; Bruce Hilton; Jeffrey Giglio; Daniel Cummings; Karl Grimm; Richard McKnight

    2009-11-01

    Correct prediction of the fission products inventory in irradiated nuclear fuels is essential for accurate estimation of fuel burnup, establishing proper requirements for spent fuel transportation and storage, materials accountability and nuclear forensics. Such prediction is impossible without accurate knowledge of neutron induced fission yields. Unfortunately, the accuracy of the fission yields reported in the ENDF/B-VII.0 library is not uniform across all of the data and much of the improvement is desired for certain isotopes and fission products. We discuss our measurements of cumulative fission yields in nuclear fuels irradiated in thermal and fast reactor spectra using Inductively Coupled Plasma Mass Spectrometry.

  8. Measurement of low radioactivity background in a high voltage cable by high resolution inductively coupled plasma mass spectrometry

    SciTech Connect

    Vacri, M. L. di; Nisi, S.; Balata, M.

    2013-08-08

    The measurement of naturally occurring low level radioactivity background in a high voltage (HV) cable by high resolution inductively coupled plasma mass spectrometry (HR ICP MS) is presented in this work. The measurements were performed at the Chemistry Service of the Gran Sasso National Laboratory. The contributions to the radioactive background coming from the different components of the heterogeneous material were separated. Based on the mass fraction of the cable, the whole contamination was calculated. The HR ICP MS results were cross-checked by gamma ray spectroscopy analysis that was performed at the low background facility STELLA (Sub Terranean Low Level Assay) of the LNGS underground lab using HPGe detectors.

  9. Gamma Ray Burst 150518a measured at different wavelengths

    NASA Astrophysics Data System (ADS)

    Apala, Ellizabeth Ann; Soderberg, Alicia Margarita; West, Michael

    2016-01-01

    Gamma Ray Burst (GRB's), extremely energetic flashes of Gamma Rays, are caused by either deaths of massive unstable stars or colliding binary neutron stars. A unique burst, GRB 150518a, had two recorded bursts fifteen minutes apart which is very rare and is considered to be ultra-long, lasting around thirty minutes total and is associated with a Supernova explosion. GBR 150518a is also extremely close compared to the average burst being measured to have a redshift of .2, this is important to note because GRB's measuring less than a redshift of .3 only are seen every ten years. Gamma rays are emitted by supernovae, neutron stars, black holes, and quasars and by studying GRB's it allows us to see more deeply into how these objects function. The first few days of GRB 150518as' detected afterglow was plotted in different wavelengths, including optical, x-ray, radio, and infrared, in flux verses time. Data is continuously being added as time goes on. This research is funded by the NSF, grant number 1358990.

  10. Resonance ionization mass spectrometry for isotopic abundance measurements

    NASA Technical Reports Server (NTRS)

    Miller, C. M.

    1986-01-01

    Resonance ionization mass spectrometry (RIMS) is a relatively new laser-based technique for the determination of isotopic abundances. The resonance ionization process depends upon the stepwise absorption of photons from the laser, promoting atoms of the element of interest through progressively higher electronic states until an ion is formed. Sensitivity arises from the efficiency of the resonant absorption process when coupled with the power available from commercial laser sources. Selectivity derives naturally from the distinct electronic structure of different elements. This isobaric discrimination has provided the major impetus for development of the technique. Resonance ionization mass spectrometry was used for analysis of the isotopic abundances of the rare earth lutetium. Isobaric interferences from ytterbium severely effect the ability to measure small amounts of the neutron-deficient Lu isotopes by conventional mass spectrometric techniques. Resonance ionization for lutetium is performed using a continuous-wave laser operating at 452 nm, through a sequential two-photon process, with one photon exciting the intermediate resonance and the second photon causing ionization. Ion yields for microgram-sized quantities of lutetium lie between 10(6) and 10(7) ions per second, at overall ionization efficiencies approaching 10(-4). Discrimination factors against ytterbium greater than 10(6) have been measured. Resonance ionization for technetium is also being explored, again in response to an isobaric interference, molybdenum. Because of the relatively high ionization potential for Tc, three-photon, two-color RIMS processes are being developed.

  11. Gamma-ray scattering for fat fraction measurement

    NASA Astrophysics Data System (ADS)

    Shakeshaft, J.; Morgan, H. M.; Lillicrap, S. C.

    1997-07-01

    The work reported examines the potential of using gamma-ray photon backscatter information to measure in vivo the percentage of fat in specific tissue volumes. gamma rays are used as the source and the backscatter detected with a hyperpure germanium detector, with ethanol (approximately 80% fat, 20% muscle) and water (muscle) being used as tissue substitutes. Two measurement techniques are examined; the measurement of the ratio of coherent scatter to Compton scatter and the measurement of the Compton scatter profile. Both are shown to be sensitive to the composition difference between ethanol and water. For the coherent - Compton scatter ratio, the measured difference between water and ethanol is 1.85:1, close to the value calculated (about 2:1). A similar difference in the coherent - Compton ratios between muscle and fat is calculated (2.2:1). The FWHM of the Compton profile has also been shown to vary with tissue composition with a difference of 0.10 keV (5%) between the ethanol and water profile widths.

  12. Thermodynamic Activity Measurements with Knudsen Cell Mass Spectrometry

    NASA Technical Reports Server (NTRS)

    Copland, Evan H.; Jacobson, Nathan S.

    2001-01-01

    Coupling the Knudsen effusion method with mass spectrometry has proven to be one of the most useful experimental techniques for studying the equilibrium between condensed phases and complex vapors. The Knudsen effusion method involves placing a condensed sample in a Knudsen cell, a small "enclosure", that is uniformly heated and held until equilibrium is attained between the condensed and vapor phases. The vapor is continuously sampled by effusion through a small orifice in the cell. A molecular beam is formed from the effusing vapor and directed into a mass spectrometer for identification and pressure measurement of the species in the vapor phase. Knudsen cell mass spectrometry (KCMS) has been used for nearly fifty years now and continues to be a leading technique for obtaining thermodynamic data. Indeed, much of the well-established vapor specie data in the JANAF tables has been obtained from this technique. This is due to the extreme versatility of the technique. All classes of materials can be studied and all constituents of the vapor phase can be measured over a wide range of pressures (approximately 10(exp -4) to 10(exp -11) bar) and temperatures (500-2800 K). The ability to selectively measure different vapor species makes KCMS a very powerful tool for the measurement of component activities in metallic and ceramic solutions. Today several groups are applying KCMS to measure thermodynamic functions in multicomponent metallic and ceramic systems. Thermodynamic functions, especially component activities, are extremely important in the development of CALPHAD (Calculation of Phase Diagrams) type thermodynamic descriptions. These descriptions, in turn, are useful for modeling materials processing and predicting reactions such as oxide formation and fiber/matrix interactions. The leading experimental methods for measuring activities are the Galvanic cell or electro-motive force (EMF) technique and the KCMS technique. Each has specific advantages, depending on

  13. Low Level Gamma Spectroscopy Measurements of Radium and Cesium in Lucerne (Medicago Sativa)

    NASA Astrophysics Data System (ADS)

    Fokapić, S.; Bikit, I.; Mrđa, D.; Vesković, M.; Slivka, J.; Mihaljev, Ž.; Ćupić, Ž.

    2007-04-01

    Nineteen years after Chernobyl nuclear accident, activity concentration of 137Cs still could be detected in food and soil samples in Central and Eastern Europe. In this paper radiation levels of radium and cesium in Lucerne will be presented. It is a perennial plant with a deep root system and it is widely grown throughout the world as forage for cattle. The samples of Lucerne were taken from twelve different locations in Vojvodina in the summer period July-September 2004. The samples were specially dried on the air and after that ground, powdered and mineralized by method of dry burning on the temperature of 450°C. Gamma spectrometry measurements of the ash were performed by means of actively shielded germanium detector with maximal background reduction. For cesium 137Cs 10 mBq/kg order of magnitude detection limits were achieved.

  14. Low Level Gamma Spectroscopy Measurements of Radium and Cesium in Lucerne (Medicago Sativa)

    SciTech Connect

    Fokapic, S.; Bikit, I.; Mrda, D.; Veskovic, M.; Slivka, J.; Mihaljev, Z.; Cupic, Z.

    2007-04-23

    Nineteen years after Chernobyl nuclear accident, activity concentration of 137Cs still could be detected in food and soil samples in Central and Eastern Europe. In this paper radiation levels of radium and cesium in Lucerne will be presented. It is a perennial plant with a deep root system and it is widely grown throughout the world as forage for cattle. The samples of Lucerne were taken from twelve different locations in Vojvodina in the summer period July-September 2004. The samples were specially dried on the air and after that ground, powdered and mineralized by method of dry burning on the temperature of 450 deg. C. Gamma spectrometry measurements of the ash were performed by means of actively shielded germanium detector with maximal background reduction. For cesium 137Cs 10 mBq/kg order of magnitude detection limits were achieved.

  15. Construction and testing of a neutron and gamma spectrometry system using pulse shape discrimination with an organic scintillator

    NASA Astrophysics Data System (ADS)

    Pope, Robert S.

    1993-03-01

    The goal of this thesis was to construct and test a neutron detector to measure the energy spectrum of 1 to 14-MeV neutrons in the presence of gammas. A spectrometer based on the process of pulse shape discrimination (PSD) was constructed, in which the scintillator NE-213 was used. The primary neutron/gamma sources used were 78-mCi and 4.7-Ci Pu-239Be sources, while 4.7-micro-Ci and 97.6-micro-Ci Na-22 gamma sources were used for energy calibration and additional testing of the detector. Proton recoil spectra and Compton electron spectra were unfolded with the neutron and gamma unfolding code FORIST to generate the incident neutron and gamma spectra, respectively. FORIST, which was written for a CDC computer, was modified to run on a VAX 6420. The experimental spectra were compared to those in the literature. The locations of the peaks in the Pu-239Be spectrum agreed with the literature to within 8.3%, the Pu-239Be gamma spectrum agreed to within 0.7%, while the Na-22 gamma spectrum agreed exactly. Uncertainties in the detection system and unfolding procedure are on the order of 5-10%. This thesis is intended to be a summary of the relevant literature and a user's guide to the PSD spectrometer.

  16. RADSAT Benchmarks for Prompt Gamma Neutron Activation Analysis Measurements

    SciTech Connect

    Burns, Kimberly A.; Gesh, Christopher J.

    2011-07-01

    The accurate and efficient simulation of coupled neutron-photon problems is necessary for several important radiation detection applications. Examples include the detection of nuclear threats concealed in cargo containers and prompt gamma neutron activation analysis for nondestructive determination of elemental composition of unknown samples. High-resolution gamma-ray spectrometers are used in these applications to measure the spectrum of the emitted photon flux, which consists of both continuum and characteristic gamma rays with discrete energies. Monte Carlo transport is the most commonly used simulation tool for this type of problem, but computational times can be prohibitively long. This work explores the use of multi-group deterministic methods for the simulation of coupled neutron-photon problems. The main purpose of this work is to benchmark several problems modeled with RADSAT and MCNP to experimental data. Additionally, the cross section libraries for RADSAT are updated to include ENDF/B-VII cross sections. Preliminary findings show promising results when compared to MCNP and experimental data, but also areas where additional inquiry and testing are needed. The potential benefits and shortcomings of the multi-group-based approach are discussed in terms of accuracy and computational efficiency.

  17. Multipurpose Radiation Resistant Semiconductor Detectors for Alpha, Neutron & Low Energy Gamma Ray Measurements at High Temperatures in High-Intensity Gamma Ray

    SciTech Connect

    Ruddy, Frank H.

    2005-06-01

    Work scheduled under year two of DOE Grant DE-FG02-04ER63734 is on schedule and all year-two milestones have or will be met. Results to date demonstrate that unprecedented silicon carbide (SiC) energy resolution has been obtained, and that SiC detectors may achieve energy resolution that exceeds that obtainable with the best silicon alpha spectrometers. Fast-neutron energy spectrometry measurements indicate that recoil-ion energy spectrometry should be possible with SiC detectors. Furthermore, SiC detectors have been demonstrated to perform well even after gamma-ray exposures of 1.E09 Rad. This result and the previously demonstrated capability of SiC detectors to operate in elevated-temperature environments are very promising for potential DOE EMSP applications. A new class of multipurpose, radiation-resistant semiconductor detectors that can be used in elevated-temperature and high-radiation environments is being developed under this grant. These detectors, based on silicon carbide (SiC) semiconductor are designed to have larger active volumes than previously available SiC detectors, and are being tested for their response to alpha particles, X-rays and low energy gamma rays, and fast neutrons.

  18. Technetium measurements by accelerator mass spectrometry at LLNL

    NASA Astrophysics Data System (ADS)

    Bergquist, B. A.; Marchetti, A. A.; Martinelli, R. E.; McAninch, J. E.; Nimz, G. J.; Proctor, I. D.; Southon, J. R.; Vogel, J. S.

    2000-10-01

    Technetium-99 is a long-lived, high-abundance fission product which has been widely distributed in the environment through atmospheric testing, the nuclear fuel cycle, and nuclear medicine. It has a high potential for migration in the environment as the pertechnetate anion. At the Center for Accelerator Mass Spectrometry, methods are being developed for the detection of this radionuclide by accelerator mass spectrometry (AMS), including extraction from environmental samples, concentration and purification of the 99Tc, conversion to a form appropriate for AMS analysis, and quantification by AMS. Besides interference from the stable (though relatively rare) atomic isobar 99Ru, the detection of 99Tc by AMS presents some technical challenges which are not present for the other radionuclides typically measured by AMS. These challenges are related to the lack of a stable Tc isotope. Here we present the status of our 99Tc methods including discussion of interferences and sensitivity, and recent results for environmental samples and the IAEA reference material IAEA-381, Irish Sea Water. Sensitivity is presently ˜10 μBq (˜1×10 8 atoms) per sample, limited primarily by 99Ru introduced from process chemicals, and precision/reproducibility is ˜15-25%.

  19. Aerosol and gamma background measurements at Basic Environmental Observatory Moussala

    NASA Astrophysics Data System (ADS)

    Angelov, Christo; Arsov, Todor; Penev, Ilia; Nikolova, Nina; Kalapov, Ivo; Georgiev, Stefan

    2016-03-01

    Trans boundary and local pollution, global climate changes and cosmic rays are the main areas of research performed at the regional Global Atmospheric Watch (GAW) station Moussala BEO (2925 m a.s.l., 42°10'45'' N, 23°35'07'' E). Real time measurements and observations are performed in the field of atmospheric chemistry and physics. Complex information about the aerosol is obtained by using a threewavelength integrating Nephelometer for measuring the scattering and backscattering coefficients, a continuous light absorption photometer and a scanning mobile particle sizer. The system for measuring radioactivity and heavy metals in aerosols allows us to monitor a large scale radioactive aerosol transport. The measurements of the gamma background and the gamma-rays spectrum in the air near Moussala peak are carried out in real time. The HYSPLIT back trajectory model is used to determine the origin of the data registered. DREAM code calculations [2] are used to forecast the air mass trajectory. The information obtained combined with a full set of corresponding meteorological parameters is transmitted via a high frequency radio telecommunication system to the Internet.

  20. Consistent Small-Sample Variances for Six Gamma-Family Measures of Ordinal Association

    ERIC Educational Resources Information Center

    Woods, Carol M.

    2009-01-01

    Gamma-family measures are bivariate ordinal correlation measures that form a family because they all reduce to Goodman and Kruskal's gamma in the absence of ties (1954). For several gamma-family indices, more than one variance estimator has been introduced. In previous research, the "consistent" variance estimator described by Cliff and colleagues…

  1. Measurement of Branching Fractions in Radiative BDecays to eta K gamma and Search for B Decays to eta' K gamma

    SciTech Connect

    Aubert, B.

    2006-03-31

    The authors present measurements of the B {yields} {eta}K{gamma} branching fractions and upper limits for the B {yields} {eta}'K{gamma} branching fractions. For B{sup +} {yields} {eta}K{sup +}{gamma} they also measure the time-integrated charge asymmetry. The data sample, collected with the BABAR detector at the Stanford Linear Accelerator Center, represents 232 x 10{sup 6} produced B{bar B} pairs. The results for branching fractions and upper limits at 90% C.L. in units of 10{sup -6} are: {Beta}(B{sup 0} {yields} {eta}K{sup 0}{gamma}) = 11.3{sub -2.6}{sup +2.8} {+-} 0.6, {Beta}(B{sup +} {yields} {eta}K{sup +}{gamma}) = 10.0 {+-} 1.3 {+-} 0.5, {Beta}(B{sup 0} {yields} {eta}'K{sup 0}{gamma}) < 6.6, {Beta}(B{sup +} {yields} {eta}'K{sup +}{gamma}) < 4.2. The charge asymmetry in the decay B{sup +} {yields} {eta}K{sup +}{gamma} is {Alpha}{sub ch} = -0.09 {+-} 0.12 {+-} 0.01. The first errors are statistical and the second systematic.

  2. Evaluation of comparison and proficiency test results of gamma ray spectrometry at Jožef Stefan Institute from 1986 to 2014.

    PubMed

    Glavič-Cindro, Denis; Korun, Matjaž; Nečemer, Marijan; Vodenik, Branko; Zorko, Benjamin

    2016-03-01

    One of the best ways to demonstrate the performance and capabilities of testing laboratories is to participate successfully in different international comparison schemes and proficiency tests. The overview of all results of such schemes in the field of high resolution gamma-ray spectrometry where the Laboratory for Radioactivity Measurements (LMR) of the Jožef Stefan Institute (JSI), Slovenia, participated in years 1986-2014 is presented. Different schemes are compared, strong points and drawbacks of different providers and schemes regarding evaluation procedures, determination of reference values, reporting time, sets of radionuclides included in the samples and range of activities of different radionuclides are discussed. One of the main conclusions is that the comparison and proficiency test samples normally contain substantially larger activities than are usually detected in environmental samples. Therefore the capability of determination of activities close to detection limits is usually covered only by few schemes.

  3. Determination of thorium-232 in Canadian soils by gamma-ray spectrometry via lead-212 and actinium-228, interference from uranium

    SciTech Connect

    Zikovsky, L.; Blagoeva, R.

    1994-12-31

    Thorium-232 background levels in non-cultivated Canadian soils (southern and northern Quebec and the Northwest Territories) are presented. Gamma-ray spectrometry was used to determine the activity of {sup 232}Th by measuring the activities of {sup 228}Ac and {sup 212}Pb at 37 sites. The specific activity levels ranged from 2.7 to 95.5 Bq/kg with an overall mean of 24.0 {+-} 15.4 Bq/kg. This activity generated an annual absorbed dose equivalent in air of 0.1 mSv. The activities of {sup 228}Ac and {sup 212}Pb in the soil increased with increasing depth. IT was found that uranium, via its decay product radium, can interfere with the determination of thorium in the soil.

  4. Direct gamma and gamma-jet measurement capability of ATLAS for Pb+Pb collisions

    SciTech Connect

    Baker, M.

    2009-12-01

    The ATLAS detector at the LHC is capable of efficiently separating photons and neutral hadrons based on their shower shapes over a wide range in {eta}, {phi}, and E{sub T}, either in addition to or instead of isolation cuts. This provides ATLAS with a unique strength for direct photon and {gamma}-jet physics as well as access to the unique capability to measure non-isolated photons from fragmentation or from the medium. We present a first look at the ATLAS direct photon measurement capabilities in Pb+Pb and, for reference, p+p collisions at {radical}s{sub NN} = 5.5 TeV over the region |{eta}| < 2.4.

  5. Low-level 14C measurements and Accelerator Mass Spectrometry

    SciTech Connect

    Litherland, A.E.; Beukens, R.P.; Zhao, X.-L.; Kieser, W.E.; Gove, H.E.

    2005-09-08

    Accelerator Mass Spectrometry (AMS) and isotope enrichment were used in 1991 to estimate that the 14C content of methane in natural gas was {<=}1.6x10-18 of the total carbon. The low content of 14C in underground hydrocarbons was verified later in the remarkable results from the Borexino test scintillation counter for solar neutrino studies. Since then studies of the 14C background problem have demonstrated that much of the background originally observed in the AMS measurements can, in principle, be eliminated. However, many difficulties and other backgrounds are to be faced as the limit for AMS is pushed still further towards possibly a ratio of < 10-21. These will be discussed.

  6. Radon potential mapping of the Tralee-Castleisland and Cavan areas (Ireland) based on airborne gamma-ray spectrometry and geology.

    PubMed

    Appleton, J D; Doyle, E; Fenton, D; Organo, C

    2011-06-01

    The probability of homes in Ireland having high indoor radon concentrations is estimated on the basis of known in-house radon measurements averaged over 10 km × 10 km grid squares. The scope for using airborne gamma-ray spectrometer data for the Tralee-Castleisland area of county Kerry and county Cavan to predict the radon potential (RP) in two distinct areas of Ireland is evaluated in this study. Airborne data are compared statistically with in-house radon measurements in conjunction with geological and ground permeability data to establish linear regression models and produce radon potential maps. The best agreement between the percentage of dwellings exceeding the reference level (RL) for radon concentrations in Ireland (% > RL), estimated from indoor radon data, and modelled RP in the Tralee-Castleisland area is produced using models based on airborne gamma-ray spectrometry equivalent uranium (eU) and ground permeability data. Good agreement was obtained between the % > RL from indoor radon data and RP estimated from eU data in the Cavan area using terrain specific models. In both areas, RP maps derived from eU data are spatially more detailed than the published 10 km grid map. The results show the potential for using airborne radiometric data for producing RP maps.

  7. Factors influencing in situ gamma-ray measurements

    NASA Astrophysics Data System (ADS)

    Loonstra, E. H.; van Egmond, F. M.

    2009-04-01

    Introduction In situ passive gamma-ray sensors are very well suitable for mapping physical soil properties. In order to make a qualitative sound soil map, high quality input parameters for calibration are required. This paper will focus on the factors that affect the output of in situ passive gamma-ray sensors, the primary source, soil, not taken into account. Factors The gamma-ray spectrum contains information of naturally occurring nuclides 40K, 238U and 232Th and man-made nuclides like 137Cs, as well as the total count rate. Factors that influence the concentration of these nuclides and the count rate can be classified in 3 categories. These are sensor design, environmental conditions and operational circumstances. Sensor design The main elements of an in situ gamma-ray sensor that influence the outcome and quality of the output are the crystal and the spectrum analysis method. Material and size of the crystal determine the energy resolution. Though widely used, NaI crystals are not the most efficient capturer of gamma radiation. Alternatives are BGO and CsI. BGO has a low peak resolution, which prohibits use in cases where man-made nuclides are subject of interest. The material is expensive and prone to temperature instability. CsI is robust compared to NaI and BGO. The density of CsI is higher than NaI, yielding better efficiency, especially for smaller crystal sizes. More volume results in higher energy efficiency. The reduction of the measured spectral information into concentration of radionuclides is mostly done using the Windows analysis method. In Windows, the activities of the nuclides are found by summing the intensities of the spectrum found in a certain interval surrounding a peak. A major flaw of the Windows method is the limited amount of spectral information that is incorporated into the analysis. Another weakness is the inherent use of ‘stripping factors' to account for contributions of radiation from nuclide A into the peak of nuclide B. This

  8. Electric Field Change Measurements of a Terrestrial Gamma Ray Flash

    NASA Astrophysics Data System (ADS)

    Marshall, Thomas; Karunarathne, Sumedhe; Stolzenburg, Maribeth

    2016-04-01

    Cummer et al. [GRL, 2014] reported on two terrestrial gamma ray flashes (TGFs) detected by the Gamma ray Burst Monitor (GBM) on the Fermi satellite. At a range of 632 km we detected an electric field change pulse associated with the first of these TGFs. The sensor bandwidth was 0.16 Hz - 2.6 MHz and was sampled at 5 MS/s. The measured zero-to-peak amplitude was 3.1 V/m. Assuming a 1/R range dependence, the amplitude range normalized to 100 km would be about 20 V/m. However, a little more than half of the path from the TGF to the sensor was over land rather than ocean, which should cause the attenuation to be greater than 1/R. Based on recent measurements of Kolmasova et al. (2015 AGU Fall Meeting), we estimate that the real peak amplitude was 40 - 50 V/m. The detected pulse was bipolar with a leading positive peak and had an overall duration of about 50 μs; these characteristics are typical of initial breakdown pulses (IBPs) that occur at the beginning of intracloud (IC) flashes. However, the pulse amplitude is an order of magnitude larger than typical IBPs. These data support the notion that IBPs of IC flashes cause TGFs [e.g., Shao et al., JGR 2010; Lu et al., GRL 2010; Cummer et al., GRL 2014].

  9. The Locations of Gamma-Ray Bursts Measured by Comptel

    NASA Technical Reports Server (NTRS)

    Kippen, R. Marc; Ryan, James M.; Connors, Alanna; Hartmann, Dieter H.; Winkler, Christoph; Kuiper, Lucien; Varendorff, Martin; McConnell, Mark L.; Hurley, Kevin; Hermsen, Wim; Schoenfelder, Volker

    1998-01-01

    The COMPTEL instrument on the Compton Gamma Ray Observatory is used to measure the locations of gamma-ray bursts through direct imaging of MeV photons. In a comprehensive search, we have detected and localized 29 bursts observed between 1991 April 19 and 1995 May 31. The average location accuracy of these events is 1.25 deg (1 sigma), including a systematic error of approx. 0.5 deg, which is verified through comparison with Interplanetary Network (IPN) timing annuli. The combination of COMPTEL and IPN measurements results in locations for 26 of the bursts with an average "error box" area of only approx. 0.3 deg (1 sigma). We find that the angular distribution of COMPTEL burst locations is consistent with large-scale isotropy and that there is no statistically significant evidence of small-angle autocorrelations. We conclude that there is no compelling evidence for burst repetition since no more than two of the events (or approx. 7% of the 29 bursts) could possibly have come from the same source. We also find that there is no significant correlation between the burst locations and either Abell clusters of galaxies or radio-quiet quasars. Agreement between individual COMPTEL locations and IPN annuli places a lower limit of approx. 100 AU (95% confidence) on the distance to the stronger bursts.

  10. Gamma rays and supernova explosions. [high temperature radiation measurement

    NASA Technical Reports Server (NTRS)

    Arnett, W. D.

    1977-01-01

    Thermal radiation associated with the explosion of supernovae is investigated. High temperature is required to produce copious gamma radiation of this sort. It appears that type 11 supernovae do not release much of their energy as gamma ray continuum radiation.

  11. Pile-up reconstruction algorithm for high count rate gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Petrovič, T.; Vencelj, M.; Lipoglavšek, M.; Novak, R.; Savran, D.

    2013-04-01

    In high count rate γ-ray spectrometry, the pile-up phenomenon turns out to be an important problem with respect to energy resolution and detection efficiency. Pile-up effects occur when two events are detected so close in time that instrumentation cannot properly extract information from both of them. Because this kind of data is incorrect and marginally useful, such data had to be rejected in traditional pulse processors. In times of digital pulse processing however, one can reconstruct piled-up pulse amplitudes by special algebraic approaches. In fully digital signal acquisition, the moving window deconvolution (MWD) method is commonly used. This method requires two parameters to be carefully set, namely the flattop time (dictated by the maximum rise time of the signal) and the shaping time, to accomplish the best possible energy resolution. In this way, the maximum energy resolution is accomplished, but a lot of piled-up events are rejected, reducing detection efficiency. We propose a method that restores some of the pile-up events, using a parallel block MWD implementation where the shaping time parameter differs for every MWD block. Careful detection of as many true events as possible, as well as determining their exact occurrence in time (their respective timestamps) is the key in getting the most out of the measured signal. With proper analysis logic we get more experimental information through reduced dead time, at the cost of controlled and selectively worsened energy resolution, on an event-by-event basis, achieving better overall detection efficiency. This method was tested on real experimental data where the detection efficiency of our method is higher, by a factor of 4.4(9), than the efficiency of a standard method with pile-up rejection at 500 kcps count rate.

  12. Radionuclide measurements by accelerator mass spectrometry at Arizona

    NASA Technical Reports Server (NTRS)

    Jull, A. J. T.; Donahue, D. J.; Zabel, T. H.

    1986-01-01

    Over the past years, Tandem Accelerator Mass Spectrometry (TAMS) has become established as an important method for radionuclide analysis. In the Arizona system the accelerator is operated at a thermal voltage of 1.8MV for C-14 analysis, and 1.6 to 2MV for Be-10. Samples are inserted into a cesium sputter ion source in solid form. Negative ions sputtered from the target are accelerated to about 25kV, and the injection magnet selects ions of a particular mass. Ions of the 3+ charge state, having an energy of about 9MeV are selected by an electrostatic deflector, surviving ions pass through two magnets, where only ions of the desired mass-energy product are selected. The final detector is a combination ionization chamber to measure energy loss (and hence, Z), and a silicon surface-barrier detector which measures residual energy. After counting the trace iosotope for a fixed time, the injected ions are switched to the major isotope used for normalization. These ions are deflected into a Faraday cup after the first high-energy magnet. Repeated measurements of the isotope ratio of both sample and standards results in a measurement of the concentration of the radionuclide. Recent improvements in sample preparation for C-14 make preparation of high-beam current graphite targets directly from CO2 feasible. Except for some measurements of standards and backgrounds for Be-10 measurements to date have been on C-14. Although most results have been in archaeology and quaternary geology, studies have been expanded to include cosmogenic C-14 in meteorites. The data obtained so far tend to confirm the antiquity of Antarctic meteorites from the Allan Hills site. Data on three samples of Yamato meteorites gave terrestrial ages of between about 3 and 22 thousand years.

  13. Measurement of Gamma Knife registered helmet factors using MOSFETs

    SciTech Connect

    Kurjewicz, Laryssa; Berndt, Anita

    2007-03-15

    The relative dose rate for the different Gamma Knife registered helmets (4, 8, 14, and 18 mm) is characterized by their respective helmet factors. Since the plateau of the dose profile for the 4 mm helmet is at most 1 mm wide, detector choices are limited. Traditionally helmet factors have been measured using 1x1x1 mm{sup 3} thermoluminescent dosimeters (TLDs). However, these are time-consuming, cumbersome measurements. This article investigates the use of metal-oxide-semiconductor field effect transistors (MOSFETs) (active area of 0.2x0.2 mm{sup 2}) as a more accurate and convenient dosimeter. Their suitability for these measurements was confirmed by basic characterization measurements. Helmet factors were measured using both MOSFETs and the established TLD approach. A custom MOSFET cassette was designed in analogy to the Elekta TLD cassette (Elekta Instruments AB) for use with the Elekta dosimetry sphere. Although both dosimeters provided values within 3% of the manufacturer's suggestion, MOSFETs provided superior accuracy and precision, in a fraction of the time required for the TLD measurements. Thus, MOSFETs proved to be a reasonable alternative to TLDs for performing helmet factor measurements.

  14. Single orthogonal sinusoidal grating for gamma correction in digital projection phase measuring profilometry

    NASA Astrophysics Data System (ADS)

    Xiao, Yanshan; Cao, Yiping; Wu, Yingchun; Shi, Shunping

    2013-05-01

    The gamma nonlinearity of the digital projector leads to obvious phase errors in the phase measuring profilometry. Based on the Fourier spectrum analysis of the captured pattern, a robust gamma correction method is proposed in this paper. An orthogonal sinusoidal grating precoded with two different known gamma values is used to evaluate the gamma value of the pattern. The evaluated gamma value is then encoded into the computer-generated phase-shifting fringe patterns before the fringe patterns are sent to the digital projector, which makes the captured fringe patterns well-sinusoidal and alleviates the phase errors caused by the gamma nonlinearity. Compared with other gamma correction methods, only one captured pattern is needed to evaluate the gamma value without loss of the accuracy. With the proposed method, a fast and accurate three-dimensional shape measurement can be achieved using the conventional three-step phase-shifting algorithm. Experiments have verified its feasibility and validity.

  15. Gamma-spectrometric measurement of radioactivity in agricultural soils of the Lombardia region, northern Italy.

    PubMed

    Guidotti, Laura; Carini, Franca; Rossi, Riccardo; Gatti, Marina; Cenci, Roberto M; Beone, Gian Maria

    2015-04-01

    This work is part of a wider monitoring project of the agricultural soils in Lombardia, which aims to build a database of topsoil properties and the potentially toxic elements, organic pollutants and gamma emitting radionuclides that the topsoils contain. A total of 156 agricultural soils were sampled according to the LUCAS (Land Use/Cover Area frame statistical Survey) standard procedure. The aim was to provide a baseline to document the conditions present at the time of sampling. The results of the project concerning soil radioactivity are presented here. The aim was to assess the content of (238)U, (232)Th, (137)Cs and (40)K by measuring soil samples by gamma spectrometry. (238)U, (232)Th and (40)K activities range 24-231, 20-70, and 242-1434 Bq kg(-1) respectively. The geographic distribution of (238)U reflects the geophysical framework of the Lombardia region: the soils with high content of uranium are distributed for the most part in the South Alpine belt, where the presence of magmatic rocks is widespread. These soils show an higher activity of (238)U than of (232)Th. The (238)U activities become lower than (232)Th when soils are located in the plain, originating from basic sedimentary rocks. (137)Cs activity ranges 0.4-86.8 kBq m(-2). The lowest activity of (137)Cs is in the plain, whereas the highest is in the North on soils kept as lawn or pasture. The (137)Cs activity of some samples suggests the presence of accumulation processes that lead to (137)Cs enriched soils. This is the first survey of gamma emitting radionuclides in Lombardia that is based on the LUCAS standard sampling. The results from this monitoring campaign are important for the human radiation exposure and provide the zero point, which will be useful for assessing future effects due to external factors such as human activities. PMID:25636137

  16. Gamma-spectrometric measurement of radioactivity in agricultural soils of the Lombardia region, northern Italy.

    PubMed

    Guidotti, Laura; Carini, Franca; Rossi, Riccardo; Gatti, Marina; Cenci, Roberto M; Beone, Gian Maria

    2015-04-01

    This work is part of a wider monitoring project of the agricultural soils in Lombardia, which aims to build a database of topsoil properties and the potentially toxic elements, organic pollutants and gamma emitting radionuclides that the topsoils contain. A total of 156 agricultural soils were sampled according to the LUCAS (Land Use/Cover Area frame statistical Survey) standard procedure. The aim was to provide a baseline to document the conditions present at the time of sampling. The results of the project concerning soil radioactivity are presented here. The aim was to assess the content of (238)U, (232)Th, (137)Cs and (40)K by measuring soil samples by gamma spectrometry. (238)U, (232)Th and (40)K activities range 24-231, 20-70, and 242-1434 Bq kg(-1) respectively. The geographic distribution of (238)U reflects the geophysical framework of the Lombardia region: the soils with high content of uranium are distributed for the most part in the South Alpine belt, where the presence of magmatic rocks is widespread. These soils show an higher activity of (238)U than of (232)Th. The (238)U activities become lower than (232)Th when soils are located in the plain, originating from basic sedimentary rocks. (137)Cs activity ranges 0.4-86.8 kBq m(-2). The lowest activity of (137)Cs is in the plain, whereas the highest is in the North on soils kept as lawn or pasture. The (137)Cs activity of some samples suggests the presence of accumulation processes that lead to (137)Cs enriched soils. This is the first survey of gamma emitting radionuclides in Lombardia that is based on the LUCAS standard sampling. The results from this monitoring campaign are important for the human radiation exposure and provide the zero point, which will be useful for assessing future effects due to external factors such as human activities.

  17. Fundamentals of gamma-ray measurements and radiometric analyses

    SciTech Connect

    Hochel, R.C.

    1990-12-31

    There are four primary modes of radioactive decay. All can be measured using various types of detectors and are the basis of many analytical techniques and much of what we know about the nucleus and its structure. Alpha particle emission occurs mostly in heavy nuclei of atomic number, Z, greater than 82 like Po, Ra, Th, and U, etc. Beta particles are simply electrons. They are emitted from the nucleus with a distribution of energies ranging from 0--3 MeV. Gamma-rays are photons with energies ranging from a few keV to 10 MeV or more. They usually follow alpha or beta decay, and depending on their energy, can have considerable range in matter. Neutrons are emitted in fission processes and also from a few of the highly excited fission product nuclei. Fission neutrons typically have energies of 1--2 MeV. Like gamma-rays, they have long ranges. The energies involved in nuclear decay processes are much higher than anything encountered in, say, chemical reactions. They are at the very top of the electromagnetic spectrum -- about a million times more energetic than visible light. As a result, these particles always produce ionization, either directly or indirectly, as they pass through matter. It is this ionization which is the basis of all radiation detectors.

  18. Fundamentals of gamma-ray measurements and radiometric analyses

    SciTech Connect

    Hochel, R.C.

    1990-01-01

    There are four primary modes of radioactive decay. All can be measured using various types of detectors and are the basis of many analytical techniques and much of what we know about the nucleus and its structure. Alpha particle emission occurs mostly in heavy nuclei of atomic number, Z, greater than 82 like Po, Ra, Th, and U, etc. Beta particles are simply electrons. They are emitted from the nucleus with a distribution of energies ranging from 0--3 MeV. Gamma-rays are photons with energies ranging from a few keV to 10 MeV or more. They usually follow alpha or beta decay, and depending on their energy, can have considerable range in matter. Neutrons are emitted in fission processes and also from a few of the highly excited fission product nuclei. Fission neutrons typically have energies of 1--2 MeV. Like gamma-rays, they have long ranges. The energies involved in nuclear decay processes are much higher than anything encountered in, say, chemical reactions. They are at the very top of the electromagnetic spectrum -- about a million times more energetic than visible light. As a result, these particles always produce ionization, either directly or indirectly, as they pass through matter. It is this ionization which is the basis of all radiation detectors.

  19. Measuring Cosmological Parameters with Gamma-Ray Bursts

    NASA Astrophysics Data System (ADS)

    Amati, Lorenzo; Valle, Massimo Della

    2015-01-01

    Gamma-Ray Bursts (GRB) emit in a few dozen of seconds up to ~1054 erg, in terms of isotropic equivalent radiated energy Eiso, therefore they can be observed up to z ~ 10 and appear very promising tools to describe the expansion rate history of the Universe. In this paper we review the use of the Ep,i-Eiso correlation of Gamma-Ray Bursts to measure ΩM. We show that the present data set of GRBs, coupled with the assumption that we live in a flat universe, can provide indipendent evidence, from other probes, that ΩM~0.3. We show that current (e.g., Swift, Fermi/GBM, Konus-WIND) and next GRB experiments (e.g., CALET/GBM, SVOM, Lomonosov/UFFO, LOFT/WFM) will allow us, within a few years, to constrain ΩM and the evolution of dark energy with time, with an accuracy comparable to that currently exhibited by SNe-Ia.

  20. 137 Ba Double Gamma Decay Measurement with GAMMASPHERE

    SciTech Connect

    Merchán, E.; Moran, K.; Lister, C. J.; Chowdhury, P.; McCutchan, E. A.; Greene, J. P.; Zhu, S.; Lauritsen, T.; Carpenter, M. P.; Shearman, R.

    2015-05-28

    The study of the electromagnetic moments (EM), and decay probability, provides detailed information about nuclear wave functions. The well-know properties of EM interactions are good for extracting information about the motion of nucleons. Higher order EM processes always occur, but are usually too weak to be measured. In the case of a 0+ → 0+ transitions, where a single gamma transition is forbidden, the simultaneous emission of two γ-rays has been studied. An interesting opportunity to further investigate 2-photon emission phenomena is by using a standard 137Cs source populating, via β-decay, the Jπ = 11/2- isomeric state at 662 keV in 137Ba. In this case, two photon process can have contributions from quadrupole-quadrupole or dipole-octupole multipolarities in direct competition with the high multipolarity M4 decay. Since the yield of the double gamma decay is around six orders of magnitude less than the first order transition, very good statistics are needed in order to observe the phenomena and great care must be taken to suppress the first-order decay. The Gammasphere array is ideal since its configuration allows a good coverage of the angular distribution and the Compton events can be suppressed. Nevertheless the process to understand and eliminate the Compton background is a challenge. Geant4 simulations were carried out to help understand and correct for those factors.

  1. 137 Ba Double Gamma Decay Measurement with GAMMASPHERE

    DOE PAGES

    Merchán, E.; Moran, K.; Lister, C. J.; Chowdhury, P.; McCutchan, E. A.; Greene, J. P.; Zhu, S.; Lauritsen, T.; Carpenter, M. P.; Shearman, R.

    2015-05-28

    The study of the electromagnetic moments (EM), and decay probability, provides detailed information about nuclear wave functions. The well-know properties of EM interactions are good for extracting information about the motion of nucleons. Higher order EM processes always occur, but are usually too weak to be measured. In the case of a 0+ → 0+ transitions, where a single gamma transition is forbidden, the simultaneous emission of two γ-rays has been studied. An interesting opportunity to further investigate 2-photon emission phenomena is by using a standard 137Cs source populating, via β-decay, the Jπ = 11/2- isomeric state at 662 keVmore » in 137Ba. In this case, two photon process can have contributions from quadrupole-quadrupole or dipole-octupole multipolarities in direct competition with the high multipolarity M4 decay. Since the yield of the double gamma decay is around six orders of magnitude less than the first order transition, very good statistics are needed in order to observe the phenomena and great care must be taken to suppress the first-order decay. The Gammasphere array is ideal since its configuration allows a good coverage of the angular distribution and the Compton events can be suppressed. Nevertheless the process to understand and eliminate the Compton background is a challenge. Geant4 simulations were carried out to help understand and correct for those factors.« less

  2. Multiphase flow measurement using multiple energy gamma ray absorption (MEGRA) composition measurement

    SciTech Connect

    Scheers, A.M.; Slijkerman, W.F.J.

    1996-12-31

    Some multiphase flowmeters use the principle of Dual Energy Gamma Ray Absorption (DEGRA) composition measurement to determine the individual water, oil and gas fractions. Under homogeneous flow conditions the ultimate uncertainty in phase fractions achievable with this technique depends strongly on the choice of hardware. The meter presented in this paper uses unique components that have been optimized for the water, oil and gas fraction measurement with theoretical uncertainties of 2% in the fractions over a 1 second measurement period. Generally, composition meters are sensitive to a change in production water salinity and this will cause significant systematic effort in the fraction and watercut measurements. A new measurement concept is presented that is not sensitive to salinity variations and based on Multiple Energy Gamma Ray Absorption (MEGRA) composition measurement. A multiphase flowmeter equipped with the MEGRA concept does not require field-calibration, a decisive advantage in subsea or marginal field developments.

  3. Determination of (241)Pu by the method of disturbed radioactive equilibrium using 2πα-counting and precision gamma-spectrometry.

    PubMed

    Alekseev, I; Kuzmina, T

    2016-04-01

    A simple technique is proposed for the determination of the content of (241)Pu, which is based on disturbance of radioactive equilibrium in the genetically related (237)U←(241)Pu→(241)Am decay chain of radionuclides, with the subsequent use of 2πα-counting and precision gamma-spectroscopy for monitoring the process of restoration of that equilibrium. It has been shown that the data on dynamics of accumulation of the daughter (241)Am, which were obtained from the results of measurements of α- and γ-spectra of the samples, correspond to the estimates calculated for the chain of two genetically related radionuclides, the differences in the estimates of (241)Pu radioactivity not exceeding 2%. Combining the different methods of registration (2πα-counting, semiconductor alpha- and gamma-spectrometry) enables the proposed method to be efficiently applied both for calibration of (241)Pu-sources (from several hundreds of kBq and higher) and for radioisotopic analysis of plutonium mixtures. In doing so, there is a deep purification of (241)Pu from its daughter decay products required due to unavailability of commercial detectors that could make it possible, based only on analysis of alpha-spectra, to conduct quantitative analysis of the content of (238)Pu and (241)Am. PMID:26868275

  4. Determination of (241)Pu by the method of disturbed radioactive equilibrium using 2πα-counting and precision gamma-spectrometry.

    PubMed

    Alekseev, I; Kuzmina, T

    2016-04-01

    A simple technique is proposed for the determination of the content of (241)Pu, which is based on disturbance of radioactive equilibrium in the genetically related (237)U←(241)Pu→(241)Am decay chain of radionuclides, with the subsequent use of 2πα-counting and precision gamma-spectroscopy for monitoring the process of restoration of that equilibrium. It has been shown that the data on dynamics of accumulation of the daughter (241)Am, which were obtained from the results of measurements of α- and γ-spectra of the samples, correspond to the estimates calculated for the chain of two genetically related radionuclides, the differences in the estimates of (241)Pu radioactivity not exceeding 2%. Combining the different methods of registration (2πα-counting, semiconductor alpha- and gamma-spectrometry) enables the proposed method to be efficiently applied both for calibration of (241)Pu-sources (from several hundreds of kBq and higher) and for radioisotopic analysis of plutonium mixtures. In doing so, there is a deep purification of (241)Pu from its daughter decay products required due to unavailability of commercial detectors that could make it possible, based only on analysis of alpha-spectra, to conduct quantitative analysis of the content of (238)Pu and (241)Am.

  5. Nondestructive and quantitative characterization of TRU and LLW mixed-waste using active and passive gamma-ray spectrometry and computed tomography

    SciTech Connect

    Camp, D.C.; Martz, H.E.

    1991-11-12

    The technology being proposed by LLNL is an Active and Passive Computed Tomography (A P CT) Drum Scanner for contact-handled (CH) wastes. It combines the advantages offered by two well-developed nondestructive assay technologies: gamma-ray spectrometry and computed tomography (CT). Coupled together, these two technologies offer to nondestructively and quantitatively characterize mixed- wastes forms. Gamma-ray spectroscopy uses one or more external radiation detectors to passively and nondestructively measure the energy spectrum emitted from a closed container. From the resulting spectrum one can identify most radioactivities detected, be they transuranic isotopes, mixed-fission products, activation products or environmental radioactivities. Spectral libraries exist at LLNL for all four. Active (A) or transmission CT is a well-developed, nondestructive medical and industrial technique that uses an external-radiation beam to map regions of varying attenuation within a container. Passive (P) or emission CT is a technique mainly developed for medical application, e.g., single-photon emission CT. Nondestructive industrial uses of PCT are under development and just coming into use. This report discuses work on the A P CT Drum Scanner at LLNL.

  6. FemtoMolar measurements using accelerator mass spectrometry.

    PubMed

    Salehpour, Mehran; Forsgard, Niklas; Possnert, Göran

    2009-03-01

    Accelerator mass spectrometry (AMS) is an ultra-sensitive analytical method suitable for the detection of sub-nM concentrations of labeled biological substances such as pharmaceutical drugs in body fluids. A limiting factor in extending the concentration measurements to the sub-pM range is the natural (14)C content in living tissues. This was circumvented by separating the labeled drug from the tissue matrix, using standard high-performance liquid chromatography (HPLC) procedures. As the separated total drug amount is in the few fg range, it is not possible to use a standard AMS sample preparation method, where mg sizes are required. We have utilized a sensitive carbon carrier method where a (14)C-deficient compound is added to the HPLC fractions and the composite sample is prepared and analyzed by AMS. Using 50 microL human blood plasma aliquots, we have demonstrated concentration measurements below 20 fM, containing sub-amol amounts of the labeled drug. The method has the immediate potential of operating in the sub-fM region. PMID:19177507

  7. Nanowire dopant measurement using secondary ion mass spectrometry

    SciTech Connect

    Chia, A. C. E.; Boulanger, J. P.; Wood, B. A.; LaPierre, R. R.; Dhindsa, N.; Saini, S. S.

    2015-09-21

    A method is presented to improve the quantitative determination of dopant concentration in semiconductor nanowire (NW) arrays using secondary ion mass spectrometry (SIMS). SIMS measurements were used to determine Be dopant concentrations in a Be-doped GaAs thin film and NW arrays of various pitches that were dry-etched from the same film. A comparison of these measurements revealed a factor of 3 to 12 difference, depending on the NW array pitch, between the secondary Be ion yields of the film and the NW arrays, despite being identically doped. This was due to matrix effects and ion beam mixing of Be from the NWs into the surrounding benzocyclobutene that was used to fill the space between the NWs. This indicates the need for etched NWs to be used as doping standards instead of 2D films when evaluating NWs of unknown doping by SIMS. Using the etched NWs as doping standards, NW arrays of various pitches grown by the vapour-liquid-solid mechanism were characterized by SIMS to yield valuable insights into doping mechanisms.

  8. Mathematical model of gamma-ray spectrometry borehole logging for quantitative analysis

    USGS Publications Warehouse

    Schimschal, Ulrich

    1981-01-01

    A technique for analyzing gamma-ray spectral-logging data has been developed, in which a digital computer is used to calculate the effects of gamma-ray attentuation in a borehole environment. The computer model allows for the calculation of the effects of lithology, porosity, density, and the thickness of a horizontal layer of uniformly distributed radioactive material surrounding a centralized probe in a cylindrical borehole. The computer program also contains parameters for the calculation of the effects of well casing, drilling fluid, probe housing, and losses through the sodium-iodide crystal. Errors associated with the commonly used mathematical assumption of a point detector are eliminated in this model. (USGS)

  9. Measurement of the Branching Ratios Gamma(D*+s -> D+s pi0)/Gamma(D*+s ->D+s gamma) and Gamma(D*0 ->D0 pi0)/Gamma(D*0 -> D0gamma)

    SciTech Connect

    Aubert, B.; Barate, R.; Boutigny, D.; Couderc, F.; Karyotakis, Y.; Lees, J.P.; Poireau, V.; Tisserand, V.; Zghiche, A.; Grauges, E.; Palano, A.; Pappagallo, M.; Pompili, A.; Chen, J.C.; Qi, N.D.; Rong, G.; Wang, P.; Zhu, Y.S.; Eigen, G.; Ofte, I.; Stugu, B. /Bergen U. /LBL, Berkeley /UC, Berkeley /Birmingham U. /Ruhr U., Bochum /Bristol U. /British Columbia U. /Brunel U. /Novosibirsk, IYF /UC, Irvine /UCLA /UC, Riverside /UC, San Diego /UC, Santa Barbara /UC, Santa Cruz /Caltech /Cincinnati U. /Colorado U. /Colorado State U. /Dortmund U. /Dresden, Tech. U. /Ecole Polytechnique /Edinburgh U. /Ferrara U. /INFN, Ferrara /Frascati /Genoa U. /INFN, Genoa /Harvard U. /Heidelberg U. /Imperial Coll., London /Iowa U. /Iowa State U. /Orsay, LAL /LLNL, Livermore /Liverpool U. /Queen Mary, U. of London /Royal Holloway, U. of London /Louisville U. /Manchester U. /Maryland U. /Massachusetts U., Amherst /MIT, LNS /McGill U. /Milan U. /INFN, Milan /Mississippi U. /Montreal U. /Mt. Holyoke Coll. /Naples U. /INFN, Naples /NIKHEF, Amsterdam /Notre Dame U. /Ohio State U. /Oregon U. /INFN, Padua /Padua U. /Paris U., VI-VII /Pennsylvania U. /Perugia U. /INFN, Perugia /Pisa U. /Pisa, Scuola Normale Superiore /INFN, Pisa /Prairie View A-M /Princeton U. /Rome U. /INFN, Rome /Rostock U. /Rutherford /DAPNIA, Saclay /South Carolina U. /SLAC /Stanford U., Phys. Dept. /SUNY, Albany /Tennessee U. /Texas U. /Texas U., Dallas /Turin U. /INFN, Turin /Trieste U. /INFN, Trieste /Valencia U., IFIC /Vanderbilt U. /Victoria U. /Warwick U. /Wisconsin U., Madison /Yale U.

    2005-08-23

    Data samples corresponding to the isospin-violating decay D*{sub s}{sup +} {yields} D{sub s}{sup +}{pi}{sup 0} and the decays D*{sub s}{sup +} {yields} D{sub s}{sup +}, D*{sup 0} {yields} D{sup 0}{pi}{sup 0} and D*{sup 0} {yields} D{sup 0}{gamma} are reconstructed using 90.4 fb{sup -1} of data recorded by the BABAR detector at the PEP-II asymmetric-energy e{sup +}e{sup -} collider. The following branching ratios are extracted: {Lambda}(D*{sub s}{sup +} {yields} D{sub s}{sup +}{pi}{sup 0})/{Lambda}(D*{sub s}{sup +} {yields} D{sub s}{sup +}{gamma}) = 0.062 {+-} 0.005(stat.) {+-} 0.006(syst.) and {Lambda}(D*{sup 0} {yields} D{sup 0}{pi}{sup 0})/{Lambda}(D*{sup 0} {yields} D{sup 0}{gamma}) = 1.74 {+-} 0.02(stat.) {+-} 0.13(syst.). Both measurements represent significant improvements over present world averages.

  10. Attributes from NMIS Time Coincidence, Fast-Neutron Imaging, Fission Mapping, And Gamma-Ray Spectrometry Data

    SciTech Connect

    Swift, Alicia L; Grogan, Brandon R; Mullens, James Allen; Hayward, J P; Mihalczo, John T

    2012-01-01

    This work tests a systematic procedure for analyzing data acquired by the Nuclear Materials Identification System (NMIS) at Oak Ridge National Laboratory with fast-neutron imaging and high-purity germanium (HPGe) gamma spectrometry capabilities. NMIS has been under development by the US Department of Energy Office of Nuclear Verification since the mid-1990s, and prior to that by the National Nuclear Security Administration Y-12 National Security Complex, with NMIS having been used at Y-12 for template matching to confirm inventory and receipts. In this present work, a complete set of NMIS time coincidence, fast-neutron imaging, fission mapping, and HPGe gamma-ray spectrometry data was obtained from Monte Carlo simulations for a configuration of fissile and nonfissile materials. The data were then presented for analysis to someone who had no prior knowledge of the unknown object to accurately determine the description of the object by applying the previously-mentioned procedure to the simulated data. The best approximation indicated that the unknown object was composed of concentric cylinders: a void inside highly enriched uranium (HEU) (84.7 {+-} 1.9 wt % {sup 235}U), surrounded by depleted uranium, surrounded by polyethylene. The final estimation of the unknown object had the correct materials and geometry, with error in the radius estimates of material regions varying from 1.58% at best and 4.25% at worst; error in the height estimates varied from 2% to 12%. The error in the HEU enrichment estimate was 5.9 wt % (within 2.5{sigma} of the true value). The accuracies of the determinations could be adequate for arms control applications. Future work will apply this iterative reconstructive procedure to other unknown objects to further test and refine it.

  11. An intercomparison of gamma-spectrometry on two samples of biological origin by eight laboratories in four countries.

    PubMed

    Twining, J R

    1996-08-01

    This report gives details of the first inter-laboratory comparison of gamma-spectrometry to be run within SPERA, the South Pacific Environmental Radioactivity Association since its inauguration in 1991. Laboratories in Australia, Chile, French Polynesia and New Zealand participated in the exercise. Two 'unknown' samples of biological origin were analysed. The first was a sample of milk powder derived from IAEA reference material. This sample provided an assessment of overall accuracy of 134Cs, 137Cs and 40K determinations. The second sample consisted of dried fish flesh including natural 40K and spiked with a mixed nuclide solution containing 210Pb, 109Cd, 54Mn, 60Co and trace 133Ba. Together the samples gave information on analytical precision over a range of energies and activities. When the results were compared with the recommended values and confidence intervals of the IAEA reference material, the overall accuracy of the gamma-spectrometry analytical procedures was found to be good. The average mean values for combined laboratory data fell within the recommended value ranges for each isotope. Ninety percent of the individual laboratory isotope mean values were within two standard errors of the 95% confidence interval of the standard, 75% were within 1 s.e., and 33% of the analyses fell within the confidence interval. Technical precision was also adequate with the overall errors being of the same magnitude as that of the reference material values for each isotope with relative standard deviations of 5-10%. There was a tendency for standard deviations of the combined results to be larger than those reported or derived from individual laboratory results by a factor between 1.2-5.6. This result suggested an under-estimate of systematic errors within individual laboratories. The largest sources of error were derived from reporting and calculation of results which gave a 16% gross error rate.

  12. 102Pd(n, {gamma}) Cross Section Measurement Using DANCE

    SciTech Connect

    Hatarik, R.; Alpizar-Vicente, A. M.; Bredeweg, T. A.; Esch, E.-I.; Haight, R. C.; O'Donnell, J. M.; Reifarth, R.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wouters, J. M.; Greife, U.

    2006-03-13

    The neutron capture cross section of the proton rich nucleus 102Pd was measured with the Detector for Advanced Neutron Capture Experiments (DANCE) at the Los Alamos Neutron Science Center. The target was a 2 mg Pd foil with 78% enriched 102Pd. It was held by a 0.9 {mu}m thick Mylar bag which was selected after comparing different thicknesses of Kapton and Mylar for their scattering background. To identify the contribution of the other Pd isotopes the data of a natural Pd sample was compared to the data of the 102Pd enriched sample. A 12C sample was used to determine the scattering background. The 102Pd(n, {gamma}) rate is of importance for the p-process nucleosynthesis.

  13. New Measurements of the Angle Gamma at the BabarExperiment

    SciTech Connect

    Orimoto, Toyoko Jennifer; /LBL, Berkeley

    2007-11-07

    Measuring the angle {gamma} is an important part of over-constraining the Unitarity Triangle to test Standard Model predictions. There are a number of methods to measure {gamma}, and we present results on the progress made in measuring {gamma} with B meson decays, using data collected with the BABAR detector at the PEP-II asymmetric energy e{sup +}e{sup -} collider at SLAC.

  14. EGAF: Measurement and Analysis of Gamma-ray Cross Sections

    NASA Astrophysics Data System (ADS)

    Firestone, R. B.; Abusaleem, K.; Basunia, M. S.; Bečvář, F.; Belgya, T.; Bernstein, L. A.; Choi, H. D.; Escher, J. E.; Genreith, C.; Hurst, A. M.; Krtička, M.; Renne, P. R.; Révay, Zs.; Rogers, A. M.; Rossbach, M.; Siem, S.; Sleaford, B.; Summers, N. C.; Szentmiklosi, L.; van Bibber, K.; Wiedeking, M.

    2014-05-01

    The Evaluated Gamma-ray Activation File (EGAF) is the result of a 2000-2007 IAEA Coordinated Research Project to develop a database of thermal, prompt γ-ray cross sections, σγ, for all elemental and selected radioactive targets. No previous database of this kind had existed. EGAF was originally based on measurements using guided neutron beams from the Budapest Reactor on all elemental targets from Z=1-82, 90 and 92, except for He and Pm. The EGAF σγ data were published in the Database of Prompt Gamma Rays from Slow Neutron Capture for Elemental Analysis [1]. An international collaboration has formed to continue the EGAF measurements with isotopically enriched targets, derive total radiative thermal neutron cross sections, σ0, extend the σγ data from thermal to 20 MeV neutrons, compile a completed activation data file, improve sections of the Reference Input Parameter Library (RIPL) with more complete and up to date level and γ-ray data, evaluate statistical γ-ray data from reaction studies, and determine recommended neutron separations energies, Sn, for atomic mass evaluations. A new guided neutron beam facility has become available at the Garching (Munich) FRM II Reactor, and high energy neutron experimental facilities are being developed by a Berkeley area collaboration where 5-33 MeV neutron beams are available at the LBNL 88” cyclotron, 2.5 and 14 MeV beams at the University of California, Berkeley neutron generator laboratory, and high flux, 10 nṡcmṡ-2 s-1, neutron pulses available from the LLNL National Ignition Facility (NIF).

  15. Gamma-carboxylation and fragmentation of osteocalcin in human serum defined by mass spectrometry.

    PubMed

    Rehder, Douglas S; Gundberg, Caren M; Booth, Sarah L; Borges, Chad R

    2015-06-01

    Serum osteocalcin (Oc) concentration is a highly specific measure of bone turnover, but its circulating proteoform(s) have not been well defined. Based on immunological methods, the major forms are thought to be the intact polypeptide and a large N-terminal-mid molecule fragment for which there is no consensus on the precise sequence. Vitamin K-dependent gamma (γ)-carboxylated variants of Oc are also found in circulation but there have been no methods that can define how many of the three potential γ-carboxyglutamic acid (Gla) residues are γ-carboxylated or provide their relative abundances. Recent reports that uncarboxylated and partially γ-carboxylated Oc forms have hormonal function underscore the need for precise evaluation of Oc at all three potential γ-carboxylation sites. Herein, mass spectrometric immunoassay (MSIA) was used to provide qualitative and semiquantitative (relative percent abundance) information on Oc molecular variants as they exist in individual plasma and serum samples. Following verification that observable Oc proteoforms were accurately assigned and not simply ex vivo artifacts, MALDI-MSIA and ESI-MSIA were used to assess the relative abundance of Oc truncation and γ-carboxylation, respectively, in plasma from 130 patients enrolled in vitamin K supplementation trials. Human Oc was found to circulate in over a dozen truncated forms with each of these displaying anywhere from 0-3 Gla residues. The relative abundance of truncated forms was consistent and unaffected by vitamin K supplementation. In contrast, when compared with placebo, vitamin K supplementation dramatically increased the fractional abundance of Oc with three Gla residues, corresponding to a decrease in the fractional abundance of Oc with zero Gla residues. These findings unequivocally document that increased vitamin K intake reduces the uncarboxylated form of Oc. Several reports of a positive effect of vitamin K intake on insulin sensitivity in humans have shown that un

  16. Gas composition measurements in arc heated flowfields via mass spectrometry

    NASA Astrophysics Data System (ADS)

    Willey, Ronald J.; Blake, David J.

    1991-06-01

    Gas compositions for an arc heated flowfield were determined by mass spectrometry on gas samples drawn from the flowfield through a sample probe. Surveys were made across the freestream flow using sample probes made of copper and quartz. Oxygen atoms reaching the mass spectrometer ranged from 6 to 9.4 percent and was a direct function of arc heater current and resultant stream enthalpy. Likewise, mole percents of nitrogen atoms ranged from 13.5 to 19 for total enthalpies of 7.0 to 18.4 MJ/kg. Species gradients existed in both the radial and axial directions. Atomic concentrations were highest near the centerline and at the nozzle exit. A species survey was completed around a shock that was established by a copper blunt body placed in the flowfield. The results showed strong species gradients following the shock edge, with atom mole fractions highest along the shock edge. Overall, the results provide insight into gas composition by point measurements in arc heated flowfields. The results suggest that nitrogen may begin dissociating before all of the oxygen dissociates, and that past assumptions based on frozen chemistry models may be faulty.

  17. Monte Carlo Solutions for Selected Problems in Gamma-Ray Spectrometry and Nuclear Activation Analysis

    SciTech Connect

    Sima, Octavian

    2008-08-14

    A comprehensive calibration of gamma-ray spectrometers cannot be obtained purely on experimental basis. Problems like self-attenuation effects, coincidence-summing effects and non-uniform source distribution (resulting e.g. from neutron self-shielding in NAA) can be efficiently solved by Monte Carlo simulation. The application of the GESPECOR code to these problems is presented and the associated uncertainty is discussed.

  18. In situ gamma-spectrometry several years after deposition of radiocesium. II. Peak-to-valley method.

    PubMed

    Gering, F; Hillmann, U; Jacob, P; Fehrenbacher, G

    1998-12-01

    A new method is introduced for deriving radiocesium soil contaminations and kerma rates in air from in situ gamma-ray spectrometric measurements. The approach makes use of additional information about gamma-ray attenuation given by the peak-to-valley ratio, which is the ratio of the count rates for primary and forward scattered photons. In situ measurements are evaluated by comparing the experimental data with the results of Monte Carlo simulations of photon transport and detector response. The influence of photons emitted by natural radionuclides on the calculation of the peak-to-valley ratio is carefully analysed. The new method has been applied to several post-Chernobyl measurements and the results agreed well with those of soil sampling. PMID:10052678

  19. Designing a minimum-functionality neutron and gamma measurement instrument with a focus on authentication

    SciTech Connect

    Karpius, Peter J; Williams, Richard B

    2009-01-01

    During the design and construction of the Next-Generation Attribute-Measurement System, which included a largely commercial off-the-shelf (COTS), nondestructive assay (NDA) system, we realized that commercial NDA equipment tends to include numerous features that are not required for an attribute-measurement system. Authentication of the hardware, firmware, and software in these instruments is still required, even for those features not used in this application. However, such a process adds to the complexity, cost, and time required for authentication. To avoid these added authenticat ion difficulties, we began to design NDA systems capable of performing neutron multiplicity and gamma-ray spectrometry measurements by using simplified hardware and software that avoids unused features and complexity. This paper discusses one possible approach to this design: A hardware-centric system that attempts to perform signal analysis as much as possible in the hardware. Simpler processors and minimal firmware are used because computational requirements are kept to a bare minimum. By hard-coding the majority of the device's operational parameters, we could cull large sections of flexible, configurable hardware and software found in COTS instruments, thus yielding a functional core that is more straightforward to authenticate.

  20. Assessment of ambient gamma dose rate around a prospective uranium mining area of South India - A comparative study of dose by direct methods and soil radioactivity measurements

    NASA Astrophysics Data System (ADS)

    Karunakara, N.; Yashodhara, I.; Sudeep Kumara, K.; Tripathi, R. M.; Menon, S. N.; Kadam, S.; Chougaonkar, M. P.

    Indoor and outdoor gamma dose rates were evaluated around a prospective uranium mining region - Gogi, South India through (i) direct measurements using a GM based gamma dose survey meter, (ii) integrated measurement days using CaSO4:Dy based thermo luminescent dosimeters (TLDs), and (iii) analyses of 273 soil samples for 226Ra, 232Th, and 40K activity concentration using HPGe gamma spectrometry. The geometric mean values of indoor and outdoor gamma dose rates were 104 nGy h-1 and 97 nGy h-1, respectively with an indoor to outdoor dose ratio of 1.09. The gamma dose rates and activity concentrations of 226Ra, 232Th, and 40K varied significantly within a small area due to the highly localized mineralization of the elements. Correlation study showed that the dose estimated from the soil radioactivity is better correlated with that measured directly using the portable survey meter, when compared to that obtained from TLDs. This study showed that in a region having localized mineralization in situ measurements using dose survey meter provide better representative values of gamma dose rates.

  1. Fission prompt gamma-ray multiplicity distribution measurements and simulations at DANCE

    SciTech Connect

    Chyzh, A; Wu, C Y; Ullmann, J; Jandel, M; Bredeweg, T; Couture, A; Norman, E

    2010-08-24

    The nearly energy independence of the DANCE efficiency and multiplicity response to {gamma} rays makes it possible to measure the prompt {gamma}-ray multiplicity distribution in fission. We demonstrate this unique capability of DANCE through the comparison of {gamma}-ray energy and multiplicity distribution between the measurement and numerical simulation for three radioactive sources {sup 22}Na, {sup 60}Co, and {sup 88}Y. The prospect for measuring the {gamma}-ray multiplicity distribution for both spontaneous and neutron-induced fission is discussed.

  2. Activity measurements and determination of gamma-ray emission intensities in the decay of 65Zn.

    PubMed

    Bé, Marie-Martine

    2006-01-01

    An International EUROMET exercise, Action 721, was organized with the objective of obtaining more reliable decay data on the disintegration of 65Zn. Nine laboratories participated, sending their results relating to activity measurements and 1115-keV gamma-ray emission intensity. Participants mainly used the 4pibeta-gamma coincidence method for the activity measurement, the resulting values and uncertainty budgets are described. New gamma-ray emission intensities were also measured in this exercise and, taking into account previously published values, the intensity of the 1115-keV gamma-ray emission has been determined to be 50.22(11)%.

  3. False positivity of gamma-glutamyl transpeptidase measurement in urine.

    PubMed

    Crivellenti, Leandro Zuccolotto; Mesa, Javier Sousa; Meirelles, Adriana Érica Wilkes Burton; Borin Crivellenti, Sofia; Mireya, Edna Gomes; Canola, Julio Carlos; Hatayde, Mário Roberto; Santana, Aureo Evangelista; Dantas, Márcio; Silva, Gyl Eanes Barros

    2014-05-01

    Although enzymuria tends to be associated to renal injury, there are no studies that have evaluated the presence of the enzyme gamma-glutamyl transpeptidase (GGT) spectrophotometry in the urine using a non-nephrotoxic agent (Nerium oleander) in order to evaluate the possibility of false positive results. The urinary GGT/urinary creatinine concentration ratio (uGGT/uCr) of 10 healthy dogs was calculated and posteriorly confronted with data from clinical evaluation, hematological and serum biochemical profiles, creatinine clearance (CrC), urinalysis, urine protein/creatinine ratio (UPC), electrocardiogram, systemic blood pressure (SBP) and light and electron microscopy. The results for kidney histology, SBP, UPC and CrC were not significantly different in any of the time-points analyzed. However, uGGT/uCr was significantly higher when measured 4 hours and 24 hours after administration of N. oleander. The measurement of the urinary GGT enzyme, as performed in many studies, yielded false positive results in dogs poisoned by a non-nephrotoxic agent.

  4. Multipurpose Radiation Resistant Semiconductor Detectors for Alpha, Neutron & Low Energy Gamma Ray Measurements at High Temperatures in High-Intensity Gamma Ray

    SciTech Connect

    Ruddy, Frank H

    2005-06-01

    Work scheduled under year two of DOE Grant DE-FG02-04ER63734 is on schedule and all year-two milestones have or will be met. Results to date demonstrate that unprecedented silicon carbide (SiC) energy resolution has been obtained, and that SiC detectors may achieve energy resolution that exceeds that obtainable with the best silicon alpha spectrometers. Fast-neutron energy spectrometry measurements indicate that recoil-ion energy spectrometry should be possible with SiC detectors. Furthermore, SiC detectors have been demonstrated to perform well even after gamma-ray exposures of 1.E09 Rad. This result and the previously demonstrated capability of SiC detectors to operate in elevated-temperature environments are very promising for potential DOE EMSP applications. A new class of multipurpose, radiation-resistant semiconductor detectors that can be used in elevated-temperature and high-radiation environments is being developed under this grant.

  5. Modern aerial gamma-ray spectrometry and regional potassium map of the conterminous United States

    USGS Publications Warehouse

    Duval, Joseph S.

    1990-01-01

    The aerial gamma-ray data were obtained as part of the National Uranium Resource Evaluation (NURE) Program sponsored by the U.S. Department of Energy during the period 1975-1983. References for the Open-File Reports that describe the surveys and data collection can be found in Bendix Field Engineering Corp. (1983). The aerial surveys were flown by contractors using fixed-wing and helicopter systems with 33-50 L (liters) of thallium-activated sodium iodide (NaI (TI)) crystals. The nominal survey altitude used is 122 m. The survey lines were generally east-west with line spacings of 1.6-10 km. Tie lines were flown perpendicular to the flight lines at intervals of 16- 30 km. The data were corrected for background from aircraft contamination and cosmic rays, altitude variations, airborne 214Bi, and Compton scattering. The gamma-ray systems were calibrated using the calibrations pads at Grand Junction, Colorado (Ward, 1978 ) and the dynamic test strip at Lake Mead, Arizona (Geodata International, Inc., 1977).  

  6. Measuring doubly 13C-substituted ethane by mass spectrometry

    NASA Astrophysics Data System (ADS)

    Clog, M.; Ling, C.; Eiler, J. M.

    2012-12-01

    Ethane (C2H6) is present in non-negligible amounts in most natural gas reservoirs and is used to produce ethylene for petrochemical industries. It is one of the by-products of lipid metabolism and is the arguably simplest molecule that can manifest multiple 13C substitutions. There are several plausible controls on the relative abundances of 13C2H6 in natural gases: thermodynamically controlled homogeneous isotope exchange reactions analogous to those behind carbonate clumped isotope thermometry; inheritance from larger biomolecules that under thermal degradation to produce natural gas; mixing of natural gases that differ markedly in bulk isotopic composition; or combinations of these and/or other, less expected fractionations. There is little basis for predicting which of these will dominate in natural samples. Here, we focus on an analytical techniques that will provide the avenue for exploring these phenomena. The method is based on high-resolution gas source isotope ratio mass spectrometry, using the Thermo 253-Ultra (a new prototype mass spectrometer). This instrument achieves the mass resolution (M/Δ M) up to 27,000, permitting separation of the isobaric interferences of potential contaminants and isotopologues of an analtye or its fragments which share a cardinal mass. We present techniques to analyze several isotopologues of molecular and fragment ions of C2H6. The critical isobaric separations for our purposes include: discrimination of 13C2H6 from 13C12CDH5 at mass 32 and separation of the 13CH3 fragment from 12CH4 at mass 16, both requiring at least a mass resolution of 20000 to make an adequate measurement. Other obvious interferences are either cleanly separated (e.g., O2, O) or accounted for by peak-stripping (CH3OH on mass 32 and NH2 on mass 16). We focus on a set of measurements which constrain: the doubly-substituted isotopologue, 13C2H6, and the 13CH3/12CH3 ratio of the methyl fragment, which constrains the bulk δ 13C. Similar methods can be

  7. Gamma-Ray Bursts: New Rulers to Measure the Universe

    NASA Astrophysics Data System (ADS)

    Ghirlanda, Giancarlo; Ghisellini, Gabriele; Lazzati, Davide; Firmani, Claudio

    2004-09-01

    The best measure of the universe should be done using a standard ``ruler'' at any redshift. Type Ia supernovae (SN Ia) probe the universe up to z~1.5, while the cosmic microwave background (CMB) primary anisotropies concern basically z~1000. Apparently, gamma-ray bursts (GRBs) are all but standard candles. However, their emission is collimated, and the collimation-corrected energy correlates tightly with the frequency at which most of the radiation of the prompt is emitted, as found by Ghirlanda et al. Through this correlation we can infer the burst energy accurately enough to probe the intermediate-redshift (z<10) universe. Using the best known 15 GRBs we find very encouraging results that emphasize the cosmological GRB role. A combined fit with SN Ia yields ΩM=0.37+/-0.10 and ΩΛ=0.87+/-0.23. Assuming in addition a flat universe, the parameters are constrained to be ΩM=0.29+/-0.04 and ΩΛ=0.71+/-0.05. GRBs accomplish the role of ``missing link'' between SN Ia and CMB primary anisotropies. They can provide a new insight on the cosmic effects of dark energy, complementary to the one supplied by CMB secondary anisotropies through the integrated Sachs-Wolfe effect. The unexpected standard candle cosmological role of GRBs motivates us with the most optimistic hopes for what can be obtained when the GRB-dedicated satellite, Swift, is launched.

  8. DEVELOPMENT OF ULTRATRACE LASER SPECTROMETRY TECHNIQUES FOR MEASUREMENTS OF ARSENIC

    EPA Science Inventory


    Development of Arsenic Speciation Techniques Based on High Performance Liquid Chromatography and Atomic Fluorescence Spectrometry

    J.B. Simeonsson, H.D. Beach and D.J. Thomas
    US EPA, Office of Research and Development, National Health and Environmental Effects Resear...

  9. Using gamma-ray emission to measure areal density of ICF capsules

    SciTech Connect

    Hoffman, Nelson M; Wilson, Douglas C; Hermann, Hans W; Young, Carlton S

    2010-01-01

    Fusion neutrons streaming from a burning ICF capsule generate gamma rays via nuclear inelastic scattering in the ablator of the capsule. The intensity of gamma-ray emission is proportional to the product of the ablator areal density ('{rho}R') and the yield of fusion neutrons, so by detecting the gamma rays we can infer the ablator areal density, provided we also have a measurement of the capsule's total neutron yield. In plastic-shell capsules, for example, {sup 12}C nuclei emit gamma rays at 4.44 MeV after excitation by 14.1-MeV neutrons from D+T fusion. These gamma rays can be measured by the Gamma Reaction History (GRH) experiment being built at the National Ignition Facility (NIF). A linear error analysis indicates the chief sources of uncertainty in inferred areal density.

  10. Estimates of rates and errors for measurements of direct-. gamma. and direct-. gamma. + jet production by polarized protons at RHIC

    SciTech Connect

    Beddo, M.E.; Spinka, H.; Underwood, D.G.

    1992-08-14

    Studies of inclusive direct-{gamma} production by pp interactions at RHIC energies were performed. Rates and the associated uncertainties on spin-spin observables for this process were computed for the planned PHENIX and STAR detectors at energies between {radical}s = 50 and 500 GeV. Also, rates were computed for direct-{gamma} + jet production for the STAR detector. The goal was to study the gluon spin distribution functions with such measurements. Recommendations concerning the electromagnetic calorimeter design and the need for an endcap calorimeter for STAR are made.

  11. Thick target measurement of the 40Ca(alpha,gamma)44Ti reaction rate

    SciTech Connect

    Sheets, S A; Burke, J T; Scielzo, N D; Phair, L; Bleuel, D; Norman, E B; Grant, P G; Hurst, A M; Tumey, S; Brown, T A; Stoyer, M

    2009-02-06

    The thick-target yield for the {sup 40}Ca({alpha},{gamma}){sup 44}Ti reaction has been measured for E{sub beam} = 4.13, 4.54, and 5.36 MeV using both an activation measurement and online {gamma}-ray spectroscopy. The results of the two measurements agree. From the measured yield a reaction rate is deduced that is smaller than statistical model calculations. This implies a smaller {sup 44}Ti production in supernova compared to recently measured {sup 40}Ca({alpha},{gamma}){sup 44}Ti reaction rates.

  12. Measuring The Variability Of Gamma-Ray Sources With AGILE

    SciTech Connect

    Chen, Andrew W.; Vercellone, Stefano; Pellizzoni, Alberto; Tavani, Marco

    2005-02-21

    Variability in the gamma-ray flux above 100 MeV at various time scales is one of the primary characteristics of the sources detected by EGRET, both allowing the identification of individual sources and constraining the unidentified source classes. We present a detailed simulation of the capacity of AGILE to characterize the variability of gamma-ray sources, discussing the implications for source population studies.

  13. Detection of frozen salt in pipes using gamma-ray spectrometry of potassium self-activity

    SciTech Connect

    Grena, Roberto; Scafe, Raffaele; Pisacane, Fabrizio; Pilato, Renzo; Crescenzi, Tommaso; Mazzei, Domenico

    2010-01-15

    Solar plants that use molten salts as heat transfer fluid need careful control to avoid the freezing of the salt in the pipes; if such a problem occurs, a diagnostic instrument to localize where is the frozen salt plug and to determine its length is useful. If the salt contains potassium (as is the case of the most common mixture used in solar plants, NaNO{sub 3}/KNO{sub 3} 60/40% by weight), the gamma decay of the natural unstable isotope {sup 40}K can be exploited to detect the frozen salt in a non-invasive way. Simulations and experimental results regarding the detectability of such plugs with different masses/lengths are presented. (author)

  14. Radiometric analysis of construction materials using HPGe gamma-ray spectrometry.

    PubMed

    Khandaker, M U; Jojo, P J; Kassim, H A; Amin, Y M

    2012-11-01

    Concentrations of primordial radionuclides in common construction materials collected from the south-west coastal region of India were determined using a high-purity germanium gamma-ray spectrometer. Average specific activities (Bq kg(-1)) for (238)U((226)Ra) in cement, brick, soil and stone samples were obtained as 54 ± 13, 21 ± 4, 50 ± 12 and 46 ± 8, respectively. Respective values of (232)Th were obtained as 65 ± 10, 21 ± 3, 58 ± 10 and 57 ± 12. Concentrations of (40)K radionuclide in cement, brick, soil and stone samples were found to be 440 ± 91, 290 ± 20, 380 ± 61 and 432 ± 64, respectively. To evaluate the radiological hazards, radium equivalent activity, various hazard indices, absorbed dose rate and annual effective dose have been calculated, and compared with the literature values. Obtained data could be used as reference information to assess any radiological contamination due to construction materials in future.

  15. U and Pu Gamma-Ray Measurements of Spent Fuel Using a Gamma-Ray Mirror Band-Pass Filter

    SciTech Connect

    Ziock, Klaus-Peter; Alameda, J.B.; Brejnholt, N.F.; Decker, T.A.; Descalle, M.A.; Fernandez-Perea, M.; Hill, R.M.; Kisner, R.A.; Melin, A.M.; Patton, B.W.; Ruz, J.; Soufli, R.; Pivovaroff, M.J.

    2014-01-01

    Abstract. We report on the use of grazing incidence gamma-ray mirrors to serve as a narrow band-pass filter for advanced non-destructive analysis (NDA) of spent nuclear fuel. The purpose of the mirrors is to limit the radiation reaching a HPGe detector to narrow spectral bands around characteristic emission lines from fissile isotopes in the fuel. This overcomes the normal rate issues when performing gamma-ray NDA measurements. In a proof-of-concept experiment, a set of simple flat gamma-ray mirrors were used to directly observe the atomic florescence lines from U and Pu from spent fuel pins with the detector located in a shirt-sleeve environment. The mirrors, consisting of highly polished silicon substrates deposited with WC/SiC multilayer coatings, successfully deflected the lines of interest while the intense primary radiation beam from the fuel was blocked by a lead beam stop. The gamma-ray multilayer coatings that make the mirrors work at the gamma-ray energies used here (~ 100 keV) have been experimentally tested at energies as high as 645 keV, indicating that direct observation of nuclear emission lines from 239Pu should be possible with an appropriately designed optic and shielding configuration.

  16. Determination of the activity concentration levels of the artificial radionuclide137Cs in soil samples collected from Qatar using high-resolution gamma-ray spectrometry

    NASA Astrophysics Data System (ADS)

    Al-Sulaiti, Huda; Nasir, Tabassum; Al Mugren, K. S.; Alkhomashi, N.; Al-Dahan, N.; Al-Dosari, M.; Bradley, D. A.; Bukhari, S.; Regan, P. H.; Santawamaitre, T.; Malain, D.; Habib, A.; Al-Dosari, Hanan; Daar, Eman

    2016-09-01

    The goal of this study was to establish the first baseline measurements for radioactivity concentration of the artificial radionuclide 137Cs in soil samples collected from the Qatarian peninsula. The work focused on the determination of the activity concentrations levels of man-made radiation in 129 soil samples collected across the landscape of the State of Qatar. All the samples were collected before the most recent accident in Japan, “the 2011 Fukushima Dai-ichi nuclear power plant accident”. The activity concentrations have been measured via high-resolution gamma-ray spectrometry using a hyper-pure germanium detector situated in a low-background environment with a copper inner-plated passive lead shield. A radiological map showing the activity concentrations of 137Cs is presented in this work. The concentration wasfound to range from 0.21 to 15.41 Bq/kg. The highest activity concentration of 137Cs was observed in sample no. 26 in North of Qatar. The mean value was found to be around 2.15 ± 0.27 Bq/kg. These values lie within the expected range relative to the countries in the region. It is expected that this contamination is mainly due to the Chernobyl accident on 26 April 1986, but this conclusion cannot be confirmed because of the lack of data before this accident.

  17. Quality management in clinical application of mass spectrometry measurement systems.

    PubMed

    Vogeser, Michael; Seger, Christoph

    2016-09-01

    Thanks to highly specific analyte detection and potentially complete compensation for matrix variables based on the principle of stable isotope derivative internal standardisation, mass spectrometry methods allow the development of diagnostic tests of outstanding analytical quality. However, these features per se do not guarantee reliability of tests. A wide range of factors can introduce analytical errors and inaccuracy due to the extreme complexity of the methods involved. Furthermore, it can be expected that the application patterns of MS methods in diagnostic laboratories will change substantially during the coming years - with presumably less specialised laboratories implementing mass spectrometry. Introduction of highly automated test solutions by manufacturers will require some trade-off between operation convenience, sample throughput and analytical performance. Structured and careful quality and risk management is therefore crucial to translate the analytical power of mass spectrometry into actionable and reliable results for individual patients' care and to maintain the degree of reliability that is expected from MS methods in clinical pathology. This reflection review discusses whether particular quality assurance tools have to be applied for MS-based diagnostic tests and whether these tools are different from those applied for optical- and affinity-based standard tests. Both pre-implementation strategies and surveillance of assays with assessment of metadata in routine testing are addressed. The release of the CLSI guideline C62-A in 2014 was a substantial achievement in this context because it addresses a wide spectrum of relevant issues in quality assurance of mass spectrometry-based clinical tests. However, the translation of this best practice document into individual laboratory settings is likely to be heterogeneous.

  18. Visualization of spatial distribution of gamma-aminobutyric acid in eggplant (Solanum melongena) by matrix-assisted laser desorption/ionization imaging mass spectrometry.

    PubMed

    Goto-Inoue, Naoko; Setou, Mitsutoshi; Zaima, Nobuhiro

    2010-01-01

    We applied imaging mass spectrometry (IMS) to determine the spatial distribution of gamma-aminobutyric acid (GABA). We found that GABA had a specific localization in seeds. We also visualized various biomolecules as well as GABA with higher spatial resolution than in the previous report. Our work suggests that IMS might be a powerful tool for exploring functional food factors, investigating the specific distribution of nutrients in unused natural resources, and evaluating the quality of functional foods.

  19. A non-parametric statistical analysis in the measurement of outdoor gamma exposure to the residents around Trombay.

    PubMed

    Kumar, Ajay; Singhal, R K; Preetha, J; Rupali, K; Joshi, V M; Hegde, A G; Kushwaha, H S

    2007-01-01

    During this study, non-parametric statistical methods were used to validate the measured gamma dose rate with the calculated one, around Trombay. Portable dose rate digital gamma spectrometry system (target fieldSPEC) was used for in situ measurement of external gamma (gamma) dose rate (measured) with the range of 1 nSv/h-10 Sv/h. The activity concentration of U-238, Th-232, K-40 and Cs-137 in the soil and their respective external dose-conversion factor (nSv/h/Bq/kg) was used to evaluate the gamma dose rate (calculated). Non-parametric statistical tool like Box- and -Whisker Plot, Spearman's (rho) rank Correlation coefficient, the Wilcoxon/Mann-Whitney test and chi(2) distribution test have been applied for validation. The randomness or discrete behaviour of measured and calculated dose rate was obvious from the Box- and -Whisker Plot as mean and median of the two are not equal. The inter quartile range (Q3-Q1), which explains about the dispersion of measured and calculated dose rate were also evaluated and found to be 10 and 16 microSv/y, respectively. The linear association between the order of ranks of the two dose rates was established by using Spearman's (rho) rank correlation that showed a coefficient of R = +0.90 with the intercept +1.9, whereas Pearson's correlation was observed with a coefficient of R = +0.93 with the intercept -25.6. Wilcoxon/Mann-Whitney test shows that, medians of the calculated and the measured dose rate as significantly different under the assumption of null hypothesis and measured dose rate was made to the normal distribution by applying Z-statistics. Value of chi(2) was calculated and found to be 284.95, which was very much greater than the critical value of chi(2)(0.05) = 43.77 at a degree of freedom 30, concluding that there is a highly significant difference between the measured and calculated dose rate at 5% significance level. PMID:17545658

  20. Measurements of alpha-gamma coincidences with an optimized dual-parameter multichannel system.

    PubMed

    Jurado Vargas, M; Caro Marroyo, B; Martín Sánchez, A

    2013-12-01

    Measurements of alpha-gamma coincidences have usually been carried out using a single channel to detect alpha-particles of a given energy, and a multichannel analyser for the detection of the corresponding coincident gamma-rays. An alpha-gamma coincidence chamber coupled to the electronic chain ending with a dual-parameter multichannel analyser has been developed and optimized. This system simultaneously stores alpha-particle, gamma-ray, and alpha-gamma coincidence spectra, which allows a general analysis to be made of the degree of coincidence between each alpha-particle and each gamma-ray emission. With this technique, a two-dimensional spectrum was obtained and analysed using "contour graphics". An application to the study of the decay scheme of (241)Am is described. PMID:24140879

  1. TL detectors for gamma ray dose measurements in criticality accidents.

    PubMed

    Miljanić, Saveta; Zorko, Benjamin; Gregori, Beatriz; Knezević, Zeljka

    2007-01-01

    Determination of gamma ray dose in mixed neutron+gamma ray fields is still a demanding task. Dosemeters used for gamma ray dosimetry are usually in some extent sensitive to neutrons and their response variations depend on neutron energy i.e., on neutron spectra. Besides, it is necessary to take into account the energy dependence of dosemeter responses to gamma rays. In this work, several types of thermoluminescent detectors (TLD) placed in different holders used for gamma ray dose determination in the mixed fields were examined. Dosemeters were from three different institutions: Ruder Bosković Institute (RBI), Croatia, JoZef Stefan Institute (JSI), Slovenia and Autoridad Regulatoria Nuclear (ARN), Argentina. All dosemeters were irradiated during the International Intercomparison of Criticality Accident Dosimetry Systems at the SILENE Reactor, Valduc, June 2002. Three accidental scenarios were reproduced and in each irradiation the dosemeters were exposed placed on the front of phantom and 'free in air'. Following types of TLDs were used: 7LiF (TLD-700), CaF2:Mn and Al2O3:Mg,Y-all from RBI; CaF2:Mn from JSI and 7LiF (TLD-700) from ARN. Reported doses were compared with the reference values as well as with the values obtained from the results of all participants. The results show satisfactory agreement with other dosimetry systems used in the Intercomparison. The influence of different types of holders and applied corrections of dosemeters' readings are discussed. PMID:17369267

  2. Measurements of gamma-ray production cross sections for shielding materials of space nuclear systems

    NASA Technical Reports Server (NTRS)

    Orphan, V. J.; John, J.; Hoot, C. G.

    1972-01-01

    Measurements of secondary gamma ray production from neutron interactions have been made over the entire energy range of interest in shielding applications. The epithermal capture gamma ray yields for both resolved gamma ray lines and continuum have been measured from thermal energies to 100 KeV for natural tungsten and U-238, two important candidate shield materials in SNAP reactor systems. Data are presented to illustrate the variation of epithermal capture gamma ray yields with neutron energy. The gamma ray production cross sections from (n,xy) reactions have been measured for Fe and Al from the threshold energies for inelastic scattering to approximately 16 MeV. Typical Fe and Al cross sections obtained with high-neutron energy resolution and averaged over broad neutron-energy groups are presented.

  3. Gamma radiation measurements and Monte Carlo computations following myocardial perfusion imaging with 201Tl.

    PubMed

    Clouvas, A; Xanthos, S

    2012-12-01

    In the current study, the time-dependent retention of (201)Tl-thallous chloride (111 MBq) was measured in a 56-y-old man undergoing myocardial perfusion imaging. For 23 d following the (201)Tl injection, total-body retained activity was measured by (i) in situ gamma spectrometry using a portable high-purity germanium (HPGe) detector and (ii) ex vivo urine radioassay using a shielded HPGe detector. The time-dependent decrease in total-body activity followed a monoexponential function, exp(-0.011 t), with an excellent correlation (R(2)=0.9988) between the experimental data and the fitted values. The effective half-life, Teff, of (201)Tl (physical half-life, Tph: 72.9 h) was therefore 63 h and the biological half-life, Tb, 463 h=19.3 d, identical to those measured in the same patient in 1997 (i.e. 14 y ago). The time-dependent decrease in the urine activity concentration, which followed a monoexponential function, exp(-0.0115 t), corroborated the foregoing results. The correlation (R(2)=0.9939) between the experimental data and the fitted values was again excellent. The effective half-life, Teff, was 60.26 h and the biological half-life, Tb, 348 h=14.5 d. Monte Carlo simulation using a simple model of the patient as a unit-density cylinder filled with water and containing a uniform distribution of (201)Tl yielded photon flux results in reasonable agreement with the measured data. PMID:22611205

  4. LC circuit as a pulse-height analyser for NaI gamma spectrometry

    NASA Astrophysics Data System (ADS)

    Tsankov, L. T.; Mitev, M. G.; Lenev, Ch. B.

    2004-11-01

    An LC circuit used as anode load of a photomultiplier tube converts its output current pulse into a damped harmonically oscillating voltage. Its amplitude is not only proportional to the transferred charge but it can be also readily encoded by the count of the successive maxima it passes until it falls below a predefined voltage level. Thus, a scintillation spectrometer may be realised in a very simple way, bypassing the classical (but rather sophisticated) solutions based on pulse-shaping amplifiers and amplitude-to-digital converters. The structure, spectral response and some experiments with a 256-channel 'LC spectrometer' are discussed. A 7% energy resolution has been achieved at 662 keV (with a ∅45×40 mm NaI(Tl) crystal). Despite some uncommon features (arising from the logarithmic channel-energy dependence), this spectrometer has useful potential in at least two fields of scintillation gamma-spectroscopy-as a portable dose-rate meter or in the study of the soft component of the cosmic rays.

  5. Radiometric analysis of construction materials using HPGe gamma-ray spectrometry.

    PubMed

    Khandaker, M U; Jojo, P J; Kassim, H A; Amin, Y M

    2012-11-01

    Concentrations of primordial radionuclides in common construction materials collected from the south-west coastal region of India were determined using a high-purity germanium gamma-ray spectrometer. Average specific activities (Bq kg(-1)) for (238)U((226)Ra) in cement, brick, soil and stone samples were obtained as 54 ± 13, 21 ± 4, 50 ± 12 and 46 ± 8, respectively. Respective values of (232)Th were obtained as 65 ± 10, 21 ± 3, 58 ± 10 and 57 ± 12. Concentrations of (40)K radionuclide in cement, brick, soil and stone samples were found to be 440 ± 91, 290 ± 20, 380 ± 61 and 432 ± 64, respectively. To evaluate the radiological hazards, radium equivalent activity, various hazard indices, absorbed dose rate and annual effective dose have been calculated, and compared with the literature values. Obtained data could be used as reference information to assess any radiological contamination due to construction materials in future. PMID:22887119

  6. Fermi large area telescope measurements of the diffuse gamma-ray emission at intermediate galactic latitudes.

    PubMed

    Abdo, A A; Ackermann, M; Ajello, M; Anderson, B; Atwood, W B; Axelsson, M; Baldini, L; Ballet, J; Barbiellini, G; Bastieri, D; Baughman, B M; Bechtol, K; Bellazzini, R; Berenji, B; Blandford, R D; Bloom, E D; Bonamente, E; Borgland, A W; Bregeon, J; Brez, A; Brigida, M; Bruel, P; Burnett, T H; Caliandro, G A; Cameron, R A; Caraveo, P A; Casandjian, J M; Cecchi, C; Charles, E; Chekhtman, A; Cheung, C C; Chiang, J; Ciprini, S; Claus, R; Cohen-Tanugi, J; Conrad, J; Dereli, H; Dermer, C D; de Angelis, A; de Palma, F; Digel, S W; Di Bernardo, G; Dormody, M; do Couto e Silva, E; Drell, P S; Dubois, R; Dumora, D; Edmonds, Y; Farnier, C; Favuzzi, C; Fegan, S J; Focke, W B; Frailis, M; Fukazawa, Y; Funk, S; Fusco, P; Gaggero, D; Gargano, F; Gehrels, N; Germani, S; Giebels, B; Giglietto, N; Giordano, F; Glanzman, T; Godfrey, G; Grenier, I A; Grondin, M-H; Grove, J E; Guillemot, L; Guiriec, S; Hanabata, Y; Harding, A K; Hayashida, M; Hays, E; Hughes, R E; Jóhannesson, G; Johnson, A S; Johnson, R P; Johnson, T J; Johnson, W N; Kamae, T; Katagiri, H; Kataoka, J; Kawai, N; Kerr, M; Knödlseder, J; Kocian, M L; Kuehn, F; Kuss, M; Lande, J; Latronico, L; Longo, F; Loparco, F; Lott, B; Lovellette, M N; Lubrano, P; Madejski, G M; Makeev, A; Mazziotta, M N; McConville, W; McEnery, J E; Meurer, C; Michelson, P F; Mitthumsiri, W; Mizuno, T; Moiseev, A A; Monte, C; Monzani, M E; Morselli, A; Moskalenko, I V; Murgia, S; Nolan, P L; Nuss, E; Ohsugi, T; Okumura, A; Omodei, N; Orlando, E; Ormes, J F; Paneque, D; Panetta, J H; Parent, D; Pelassa, V; Pepe, M; Pesce-Rollins, M; Piron, F; Porter, T A; Rainò, S; Rando, R; Razzano, M; Reimer, A; Reimer, O; Reposeur, T; Ritz, S; Rodriguez, A Y; Roth, M; Ryde, F; Sadrozinski, H F-W; Sanchez, D; Sander, A; Saz Parkinson, P M; Scargle, J D; Sellerholm, A; Sgrò, C; Smith, D A; Smith, P D; Spandre, G; Spinelli, P; Starck, J-L; Stecker, F W; Striani, E; Strickman, M S; Strong, A W; Suson, D J; Tajima, H; Takahashi, H; Tanaka, T; Thayer, J B; Thayer, J G; Thompson, D J; Tibaldo, L; Torres, D F; Tosti, G; Tramacere, A; Uchiyama, Y; Usher, T L; Vasileiou, V; Vilchez, N; Vitale, V; Waite, A P; Wang, P; Winer, B L; Wood, K S; Ylinen, T; Ziegler, M

    2009-12-18

    The diffuse galactic gamma-ray emission is produced by cosmic rays (CRs) interacting with the interstellar gas and radiation field. Measurements by the Energetic Gamma-Ray Experiment Telescope (EGRET) instrument on the Compton Gamma-Ray Observatory indicated excess gamma-ray emission greater, > or approximately equal to 1 GeV relative to diffuse galactic gamma-ray emission models consistent with directly measured CR spectra (the so-called "EGRET GeV excess"). The Large Area Telescope (LAT) instrument on the Fermi Gamma-Ray Space Telescope has measured the diffuse gamma-ray emission with improved sensitivity and resolution compared to EGRET. We report on LAT measurements for energies 100 MeV to 10 GeV and galactic latitudes 10 degrees < or = |b| < or = 20 degrees. The LAT spectrum for this region of the sky is well reproduced by a diffuse galactic gamma-ray emission model that is consistent with local CR spectra and inconsistent with the EGRET GeV excess. PMID:20366246

  7. Fermi Large Area Telescope Measurements of the Diffuse Gamma-Ray Emission at Intermediate Galactic Latitudes

    SciTech Connect

    Abdo, A.A.; Ackermann, M.; Ajello, M.; Anderson, B.; Atwood, W.B.; Axelsson, M.; Baldini, L.; Ballet, J.; Barbiellini, G.; Bastieri, D.; Baughman, B.M.; Bechtol, K.; Bellazzini, R.; Berenji, B.; Blandford, R.D.; Bloom, E.D.; Bonamente, E.; Borgland, A.W.; Bregeon, J.; Brez, A.; Brigida, M.; /more authors..

    2012-04-11

    The diffuse galactic {gamma}-ray emission is produced by cosmic rays (CRs) interacting with the interstellar gas and radiation field. Measurements by the Energetic Gamma-Ray Experiment Telescope (EGRET) instrument on the Compton Gamma-Ray Observatory indicated excess {gamma}-ray emission {ge}1 GeV relative to diffuse galactic {gamma}-ray emission models consistent with directly measured CR spectra (the so-called 'EGRET GeV excess'). The Large Area Telescope (LAT) instrument on the Fermi Gamma-Ray Space Telescope has measured the diffuse {gamma}-ray emission with improved sensitivity and resolution compared to EGRET. We report on LAT measurements for energies 100 MeV to 10 GeV and galactic latitudes 10{sup o} {le} |b| {le} 20{sup o}. The LAT spectrum for this region of the sky is well reproduced by a diffuse galactic {gamma}-ray emission model that is consistent with local CR spectra and inconsistent with the EGRET GeV excess.

  8. Ground gamma-ray survey of the Solforata gas discharge area, Alban Hills-Italy: a comparison between field and laboratory measurements.

    PubMed

    Di Paolo, Federico; Plastino, Wolfango; Povinec, Pavel P; Bella, Francesco; Budano, Antonio; De Vincenzi, Mario; Laubenstein, Matthias; Ruggieri, Federico

    2013-01-01

    Measurements of environmental radioactivity by HPGe gamma-spectrometry were carried out with the aim of investigating the distribution of natural radionuclides in a volcanic area and to compare two different methodologies - an in situ gamma-survey of the area and high accuracy laboratory measurements of soil samples. Results demonstrate good performance of the in situ technique, also confirmed by a correlation analysis between the results obtained by the two methodologies. A volcanic gas discharge area was chosen as the test site for the presence of natural long-lived radionuclides such as (40)K and (238)U, (235)U and (232)Th, and their decay chain members. Clear evidence of (222)Rn degassing in the area was confirmed by (226)Ra values measured by the in situ technique. Higher (40)K values measured by the in situ technique may be attributed to the presence of vegetation in the study area. PMID:22982169

  9. Gamma-ray spectrometry of humans at the University of Utah.

    PubMed

    Lloyd, R D; Mays, C W; Taysum, D H

    1979-04-30

    A human total-body counter was designed and built with two 20 X 10 cm NaI (Tl) crystals suspended over an "isoresponse surface" upon which the subject reclines. This surface is curved from head to knee and from left to right, so that a gamma-ray emitting object is detected with equal efficiency when placed anywhere upon it. The positioner and detectors are housed in a low background enclosure constructed of steel 31 cm thick with a graded inner lining of lead + cadmium + copper. Calibration of the system was accomplished by administering trace amounts of various radionuclides to 48 human subjects of various sizes, ranging in age from 4--80 years. Counting rates per retained muCi at 0.53, 0.66, 1.53, and 2.75 MeV (83Rb, 137Cs, 42K, and 24Na) were determined as a function of body size and were compared with counting rates per muCi of corresponding emitters centered in a polyethylene cylinder of radius 10.3 cm. Limits of detection, corresponding to three times the standard deviation of a 50 min background, were 170 nCi 90Sr (via Bremsstrahlung X-rays), 0.78 nCi 131I, 0.48 nCi 83Rb, 0.52 nCi 137 Cs, 4.9 nCi 40K (or 5.8 g of natural potassium) and 1.7 nCi 222Rn. PMID:112640

  10. Multipurpose Radiation Resistant Semiconductor Detectors for Alpha, Neutron & Low Energy Gamma Ray Measurements at High Temperatures in High-Intensity Gamma Ray

    SciTech Connect

    Ruddy, Frank H.

    2005-06-01

    Work scheduled under year two of DOE Grant DE-FG02-04ER63734 is on schedule and all year-two milestones have or will be met. Results to date demonstrate that unprecedented silicon carbide (SiC) energy resolution has been obtained, and that SiC detectors may achieve energy resolution that exceeds that obtainable with the best silicon alpha spectrometers. Fast-neutron energy spectrometry measurements indicate that recoil-ion energy spectrometry should be possible with SiC detectors. Furthermore, SiC detectors have been demonstrated to perform well even after gamma-ray exposures of 1.E09 Rad. This result and the previously demonstrated capability of SiC detectors to operate in elevated-temperature environments are very promising for potential DOE EMSP applications. A new class of multipurpose, radiation-resistant semiconductor detectors that can be used in elevated-temperature and high-radiation environments is being developed under this grant. These detectors, based on silicon carbide (SiC) semiconductor are designed to have larger active volumes than previously available SiC detectors, and are being tested for their response to alpha particles, X-rays and low energy gamma rays, and fast neutrons. Specifically, SiC radiation detectors with larger areas and 100-micrometer thick active regions have been designed and manufactured according to detector-design specifications. Detectors based on a Schottky diode design were specified in order to minimize the effects of the detector entrance window on alpha particle measurements. During manufacture of the Schottky diodes, the manufacturer also provided a set of large-volume SiC p-i-n diodes for testing Extensive alpha particle measurements have been carried out to test and quantify the response of the SiC Schottky diodes. Exposures to 148-Gd, 213-Po, 217-At, 221-Fr, 225-Ac, 237-Np, 238-Pu, 240-Pu, and 242-Pu sources were used to obtain detailed alpha response data in the alpha energy range from 3182.787 keV to 8375.9 ke

  11. Assessing sample attenuation parameters for use in low-energy efficiency transfer in gamma-ray spectrometry.

    PubMed

    Bruggeman, M; Verheyen, L; Vidmar, T; Liu, B

    2016-03-01

    We present a numerical fitting method for transmission data that outputs an equivalent sample composition. This output is used as input to a generalised efficiency transfer model based on the EFFTRAN software integrated in a LIMS. The procedural concept allows choosing between efficiency transfer with a predefined sample composition or with an experimentally determined composition based on a transmission measurement. The method can be used for simultaneous quantification of low-energy gamma emitters like (210)Pb, (241)Am, (234)Th in typical environmental samples.

  12. A UK comparison for measurements of low levels of gamma-emitters in waste drums.

    PubMed

    Dean, Julian

    2009-05-01

    Much of the work of the UK nuclear industry is now concerned with decommissioning many of the existing power stations and other facilities. An important aspect of this work is the accurate measurement of low levels of radioactivity in waste forms such as building materials in order that these materials can be assigned to the correct waste streams. This has led to a call for suitable standards and reference materials, and the specific needs of UK users were identified at an NPL workshop in 2005. One of the highest priorities was for 'soft waste' spiked with gamma-emitters in a 200 L drum format, with an activity concentration of just under 0.4 Bq g(-1). In response, NPL prepared a single reference drum meeting this specification. The low density was achieved by loading the drum with plastic bottles, each partially loaded with ion-exchange resin. The resin in each bottle had been previously spiked with a mixture of (241)Am, (137)Cs and (60)Co, all traceable to national standards. The drum would be used primarily as the basis of a comparison exercise, but feedback on its usefulness as a calibration standard would also be sought. The drum was measured by 17 radioassay groups at 15 UK sites. The monitors used were mostly commercial gamma-spectrometry systems designed to accommodate waste drums. Some groups measured the drum on more than one monitor and some used more than one efficiency calibration. Many of the groups used mathematical modelling to derive their efficiencies. The results of the exercise were discussed at a second NPL workshop (2007), after which the participants were allowed to submit supplementary or replacement results (with reasons for any changes clearly stated). In total, 88 results were submitted. A total of 51 results were in agreement with the NPL values; of the remaining results, 24 were explained by the participants concerned (or were revised to provide supplementary values), but the other 13 results were either clearly discrepant or

  13. First Direct Measurement of the 17F(p,gamma)18Ne Cross Section

    SciTech Connect

    Chipps, K.; Bardayan, Daniel W; Nesaraja, Caroline D; Pain, S. D.; Smith, Michael Scott; Blackmon, Jeff C; Chae, K. Y.; Moazen, Brian; Pittman, S. T.; Greife, U.; Hatarik, Robert; Peters, W. A.; Kozub, R. L.; ShrinerJr., J. F.; Matei, Catalin

    2009-01-01

    The rate of the {sup 17}F(p,{gamma}){sup 18}Ne reaction is important in various astrophysical events. A previous {sup 17}F(p,p){sup 17}F measurement identified a 3{sup +} state providing the strongest resonance contribution, but the resonance strength was unknown. We have directly measured the {sup 17}F(p,{gamma}){sup 18}Ne reaction using a mixed beam of {sup 17}F and {sup 17}O at ORNL. The resonance strength for the 3{sup +} resonance in {sup 18}Ne was found to be {omega}{gamma} = 33 {+-} 14(stat) {+-} 17(syst) meV, corresponding to a {gamma} width of {Lambda}{sub {gamma}} = 56 {+-} 24(stat) {+-} 30(syst) meV. An upper limit on the direct capture of S(E) {le} 65 keV b was determined at an energy of 800 keV.

  14. Measurement of the direct CP asymmetry in b-->s gamma Decays.

    PubMed

    Aubert, B; Barate, R; Boutigny, D; Couderc, F; Gaillard, J M; Hicheur, A; Karyotakis, Y; Lees, J P; Tisserand, V; Zghiche, A; Palano, A; Pompili, A; Chen, J C; Qi, N D; Rong, G; Wang, P; Zhu, Y S; Eigen, G; Ofte, I; Stugu, B; Abrams, G S; Borgland, A W; Breon, A B; Brown, D N; Button-Shafer, J; Cahn, R N; Charles, E; Day, C T; Gill, M S; Gritsan, A V; Groysman, Y; Jacobsen, R G; Kadel, R W; Kadyk, J; Kerth, L T; Kolomensky, Yu G; Kukartsev, G; LeClerc, C; Lynch, G; Merchant, A M; Mir, L M; Oddone, P J; Orimoto, T J; Pripstein, M; Roe, N A; Ronan, M T; Shelkov, V G; Wenzel, W A; Ford, K; Harrison, T J; Hawkes, C M; Morgan, S E; Watson, A T; Fritsch, M; Goetzen, K; Held, T; Koch, H; Lewandowski, B; Pelizaeus, M; Steinke, M; Boyd, J T; Chevalier, N; Cottingham, W N; Kelly, M P; Latham, T E; Wilson, F F; Cuhadar-Donszelmann, T; Hearty, C; Knecht, N S; Mattison, T S; McKenna, J A; Thiessen, D; Khan, A; Kyberd, P; Teodorescu, L; Blinov, V E; Bukin, A D; Druzhinin, V P; Golubev, V B; Ivanchenko, V N; Kravchenko, E A; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Yushkov, A N; Best, D; Bruinsma, M; Chao, M; Eschrich, I; Kirkby, D; Lankford, A J; Mandelkern, M; Mommsen, R K; Roethel, W; Stoker, D P; Buchanan, C; Hartfiel, B L; Gary, J W; Shen, B C; Wang, K; del Re, D; Hadavand, H K; Hill, E J; MacFarlane, D B; Paar, H P; Rahatlou, S; Sharma, V; Berryhill, J W; Campagnari, C; Dahmes, B; Levy, S L; Long, O; Lu, A; Mazur, M A; Richman, J D; Verkerke, W; Beck, T W; Eisner, A M; Heusch, C A; Lockman, W S; Schalk, T; Schmitz, R E; Schumm, B A; Seiden, A; Spradlin, P; Williams, D C; Wilson, M G; Albert, J; Chen, E; Dubois-Felsmann, G P; Dvoretskii, A; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Ryd, A; Samuel, A; Yang, S; Jayatilleke, S; Mancinelli, G; Meadows, B T; Sokoloff, M D; Abe, T; Blanc, F; Bloom, P; Chen, S; Ford, W T; Nauenberg, U; Olivas, A; Rankin, P; Smith, J G; Zhang, J; Zhang, L; Chen, A; Harton, J L; Soffer, A; Toki, W H; Wilson, R J; Zeng, Q L; Altenburg, D; Brandt, T; Brose, J; Colberg, T; Dickopp, M; Feltresi, E; Hauke, A; Lacker, H M; Maly, E; Müller-Pfefferkorn, R; Nogowski, R; Otto, S; Petzold, A; Schubert, J; Schubert, K R; Schwierz, R; Spaan, B; Sundermann, J E; Bernard, D; Bonneaud, G R; Brochard, F; Grenier, P; Schrenk, S; Thiebaux, C; Vasileiadis, G; Verderi, M; Bard, D J; Clark, P J; Lavin, D; Muheim, F; Playfer, S; Xie, Y; Andreotti, M; Azzolini, V; Bettoni, D; Bozzi, C; Calabrese, R; Cibinetto, G; Luppi, E; Negrini, M; Piemontese, L; Sarti, A; Treadwell, E; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Patteri, P; Piccolo, M; Zallo, A; Buzzo, A; Capra, R; Contri, R; Crosetti, G; Lo Vetere, M; Macri, M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Santroni, A; Tosi, S; Bailey, S; Brandenburg, G; Morii, M; Won, E; Dubitzky, R S; Langenegger, U; Bhimji, W; Bowerman, D A; Dauncey, P D; Egede, U; Gaillard, J R; Morton, G W; Nash, J A; Taylor, G P; Grenier, G J; Mallik, U; Cochran, J; Crawley, H B; Lamsa, J; Meyer, W T; Prell, S; Rosenberg, E I; Yi, J; Davier, M; Grosdidier, G; Höcker, A; Laplace, S; Le Diberder, F; Lepeltier, V; Lutz, A M; Petersen, T C; Plaszczynski, S; Schune, M H; Tantot, L; Wormser, G; Cheng, C H; Lange, D J; Simani, M C; Wright, D M; Bevan, A J; Coleman, J P; Fry, J R; Gabathuler, E; Gamet, R; Parry, R J; Payne, D J; Sloane, R J; Touramanis, C; Back, J J; Cormack, C M; Harrison, P F; Mohanty, G B; Brown, C L; Cowan, G; Flack, R L; Flaecher, H U; Green, M G; Marker, C E; McMahon, T R; Ricciardi, S; Salvatore, F; Vaitsas, G; Winter, M A; Brown, D; Davis, C L; Allison, J; Barlow, N R; Barlow, R J; Hart, P A; Hodgkinson, M C; Lafferty, G D; Lyon, A J; Williams, J C; Farbin, A; Hulsbergen, W D; Jawahery, A; Kovalskyi, D; Lae, C K; Lillard, V; Roberts, D A; Blaylock, G; Dallapiccola, C; Flood, K T; Hertzbach, S S; Kofler, R; Koptchev, V B; Moore, T B; Saremi, S; Staengle, H; Willocq, S; Cowan, R; Sciolla, G; Taylor, F; Yamamoto, R K; Mangeol, D J J; Patel, P M; Robertson, S H; Lazzaro, A; Palombo, F; Bauer, J M; Cremaldi, L; Eschenburg, V; Godang, R; Kroeger, R; Reidy, J; Sanders, D A; Summers, D J; Zhao, H W; Brunet, S; Côté, D; Taras, P; Nicholson, H; Cavallo, N; Fabozzi, F; Gatto, C; Lista, L; Monorchio, D; Paolucci, P; Piccolo, D; Sciacca, C; Baak, M; Bulten, H; Raven, G; Wilden, L; Jessop, C P; LoSecco, J M; Gabriel, T A; Allmendinger, T; Brau, B; Gan, K K; Honscheid, K; Hufnagel, D; Kagan, H; Kass, R; Pulliam, T; Rahimi, A M; Ter-Antonyan, R; Wong, Q K; Brau, J; Frey, R; Igonkina, O; Potter, C T; Sinev, N B; Strom, D; Torrence, E; Colecchia, F; Dorigo, A; Galeazzi, F; Margoni, M; Morandin, M; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Tiozzo, G; Voci, C; Benayoun, M; Briand, H; Chauveau, J; David, P; de la Vaissière, C; Del Buono, L; Hamon, O; John, M J J; Leruste, P; Ocariz, J; Pivk, M; Roos, L; T'Jampens, S; Therin, G; Manfredi, P F; Re, V; Behera, P K; Gladney, L; Guo, Q H; Panetta, J; Anulli, F; Biasini, M; Peruzzi, I M; Pioppi, M; Angelini, C; Batignani, G; Bettarini, S; Bondioli, M; Bucci, F; Calderini, G; Carpinelli, M; Del Gamba, V; Forti, F; Giorgi, M A; Lusiani, A; Marchiori, G; Martinez-Vidal, F; Morganti, M; Neri, N; Paoloni, E; Rama, M; Rizzo, G; Sandrelli, F; Walsh, J; Haire, M; Judd, D; Paick, K; Wagoner, D E; Danielson, N; Elmer, P; Lau, Y P; Lu, C; Miftakov, V; Olsen, J; Smith, A J S; Telnov, A V; Bellini, F; Cavoto, G; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Li Gioi, L; Mazzoni, M A; Morganti, S; Pierini, M; Piredda, G; Safai Tehrani, F; Voena, C; Christ, S; Wagner, G; Waldi, R; Adye, T; De Groot, N; Franek, B; Geddes, N I; Gopal, G P; Olaiya, E O; Aleksan, R; Emery, S; Gaidot, A; Ganzhur, S F; Giraud, P F; Hamel de Monchenault, G; Kozanecki, W; Langer, M; Legendre, M; London, G W; Mayer, B; Schott, G; Vasseur, G; Yèche, C; Zito, M; Purohit, M V; Weidemann, A W; Yumiceva, F X; Aston, D; Bartoldus, R; Berger, N; Boyarski, A M; Buchmueller, O L; Convery, M R; Cristinziani, M; De Nardo, G; Dong, D; Dorfan, J; Dujmic, D; Dunwoodie, W; Elsen, E E; Fan, S; Field, R C; Glanzman, T; Gowdy, S J; Hadig, T; Halyo, V; Hast, C; Hryn'ova, T; Innes, W R; Kelsey, M H; Kim, P; Kocian, M L; Leith, D W G S; Libby, J; Luitz, S; Luth, V; Lynch, H L; Marsiske, H; Messner, R; Muller, D R; O'Grady, C P; Ozcan, V E; Perazzo, A; Perl, M; Petrak, S; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Simi, G; Snyder, A; Soha, A; Stelzer, J; Su, D; Sullivan, M K; Va'vra, J; Wagner, S R; Weaver, M; Weinstein, A J R; Wisniewski, W J; Wittgen, M; Wright, D H; Yarritu, A K; Young, C C; Burchat, P R; Edwards, A J; Meyer, T I; Petersen, B A; Roat, C; Ahmed, S; Alam, M S; Ernst, J A; Saeed, M A; Saleem, M; Wappler, F R; Bugg, W; Krishnamurthy, M; Spanier, S M; Eckmann, R; Kim, H; Ritchie, J L; Satpathy, A; Schwitters, R F; Izen, J M; Kitayama, I; Lou, X C; Ye, S; Bianchi, F; Bona, M; Gallo, F; Gamba, D; Borean, C; Bosisio, L; Cartaro, C; Cossutti, F; Della Ricca, G; Dittongo, S; Grancagnolo, S; Lanceri, L; Poropat, P; Vitale, L; Vuagnin, G; Panvini, R S; Banerjee, S; Brown, C M; Fortin, D; Jackson, P D; Kowalewski, R; Roney, J M; Band, H R; Dasu, S; Datta, M; Eichenbaum, A M; Graham, M; Hollar, J J; Johnson, J R; Kutter, P E; Li, H; Liu, R; Di Lodovico, F; Mihalyi, A; Mohapatra, A K; Pan, Y; Prepost, R; Rubin, A E; Sekula, S J; Tan, P; von Wimmersperg-Toeller, J H; Wu, J; Wu, S L; Yu, Z; Neal, H

    2004-07-01

    We describe a measurement of the direct CP asymmetry between inclusive b-->s gamma and b-->s gamma decays. This asymmetry is expected to be less than 0.01 in the standard model, but could be enhanced up to about 0.10 by new physics contributions. We use a sample of 89 x 10(6) BB pairs recorded with the BABAR detector at SLAC PEP-II, from which we reconstruct a set of 12 exclusive b-->s gamma final states containing one charged or neutral kaon and one to three pions. We measure an asymmetry of A(CP)(b-->s gamma)=0.025+/-0.050(stat)+/-0.015(syst), corresponding to an allowed range of -0.06s gamma)<+0.11 at 90% confidence level.

  15. Neutron and gamma dose and spectra measurements on the Little Boy replica

    SciTech Connect

    Hoots, S.; Wadsworth, D.

    1984-06-01

    The radiation-measurement team of the Weapons Engineering Division at Lawrence Livermore National Laboratory (LLNL) measured neutron and gamma dose and spectra on the Little Boy replica at Los Alamos National Laboratory (LANL) in April 1983. This assembly is a replica of the gun-type atomic bomb exploded over Hiroshima in 1945. These measurements support the National Academy of Sciences Program to reassess the radiation doses due to atomic bomb explosions in Japan. Specifically, the following types of information were important: neutron spectra as a function of geometry, gamma to neutron dose ratios out to 1.5 km, and neutron attenuation in the atmosphere. We measured neutron and gamma dose/fission from close-in to a kilometer out, and neutron and gamma spectra at 90 and 30/sup 0/ close-in. This paper describes these measurements and the results. 12 references, 13 figures, 5 tables.

  16. A Users' Guide for the Computer Program ISDMAP: Analysis and Mapping of In-Situ Gamma-Ray Spectrometry and Soil Sample Data

    SciTech Connect

    Reginatto, Marcel; Bailey, Paul; Shebell, Peter

    2000-11-30

    The computer program ISDMAP was written to analyze data from a set of in situ gamma-ray spectrometry measurements on a grid. It can also do a combined analysis of this type of data and data from soil samples. One well-known difficulty with attempting this type of analysis is that such sets of data can never provide enough information to determine a unique solution. This can be understood intuitively since a finite number of measurements cannot be sufficient to determine a continuous distribution (this observation is not restricted to data collected with the in situ technique, but holds for any set of discrete measurements, such as a series of soil samples). One can, however, restrict to particular types of solutions by requiring that they satisfy other conditions in addition to the measurements, and this is the approach taken by ISDMAP. In ISDMAP, the data are analyzed in a different manner depending on whether the data is from a characterization survey or from a post-remediation survey. The ''characterization'' option creates a map of contamination in surface soil that is smooth and fits the data. The ''post-remediation'' option creates a map with a summary of potential hot spots over a constant background level, providing a map of hot spots that might be ''hidden'' in the data. This report describes the operation of ISDMAP in sufficient detail to allow a user to prepare the necessary input files and run the program. The program requires a PC with DOS or a DOS emulator (most Windows machines have this).

  17. Determination of the natural radioactivity levels in north west of Dukhan, Qatar using high-resolution gamma-ray spectrometry.

    PubMed

    Al-Sulaiti, Huda; Nasir, Tabassum; Al Mugren, K S; Alkhomashi, N; Al-Dahan, N; Al-Dosari, M; Bradley, D A; Bukhari, S; Matthews, M; Regan, P H; Santawamaitre, T; Malain, D; Habib, A

    2012-07-01

    This study is aimed at the determination of the activity concentrations of naturally occuring and technologically enhanced levels of radiation in 34 representative soil samples that have been collected from an inshore oil field area which was found to have, in a previous study, the highest observed value of 226Ra concentration among 129 soil samples. The activity concentrations of 238U and 226Ra have been inferred from gamma-ray transitions associated with their decay progenies and measured using a hyper-pure germanium detector. Details of the sample preparation and the gamma-ray spectroscopic analysis techniques are presented, together with the values of the activity concentrations associated with the naturally occuring radionuclide chains for all the samples collected from NW Dukhan. Discrete-line, gamma-ray energy transitions from spectral lines ranging in energy from ∼100 keV up to 2.6 MeV have been associated with characteristic decays of the various decay products within the 235.8U and 232Th radioactive decay chains. These data have been analyzed, under the assumption of secular equilibrium for the U and Th decay chains. Details of the sample preparation and the gamma-ray spectroscopic analysis techniques are presented. The weighted mean value of the activity concentrations of 226Ra in one of the samples was found to be around a factor of 2 higher than the values obtained in the previous study and approximately a factor of 10 higher than the accepted worldwide average value of 35 Bq/kg. The weighted mean values of the activity concentrations of 232Th and 40K were also deduced and found to be within the worldwide average values of 30 and 400 Bq/kg, respectively. Our previous study reported a value of 201.9±1.5Stat.±13Syst.Bq/kg for 226Ra in one sample and further investigation in the current work determined a measured value for 226Ra of 342.00±1.9Stat.±25Syst.Bq/kg in a sample taken from the same locality. This is significantly higher than all the other

  18. Studies of charmed hadronic B decays with the early LHCb data and prospects for {gamma} measurements

    SciTech Connect

    Nardulli, J.

    2010-12-22

    We present the first studies of decays of the type B{yields}DX, where D represents a charmed meson (D{sup 0}, D{sup (*)+}, or D{sub s}) from the LHCb experiment at CERN. Our studies use data accumulated during the 2010 run of the LHC. This work represents the first steps on a programme towards a precision measurement of the angle {gamma} of the CKM Unitarity Triangle. The prospects for this {gamma} measurement will be reviewed.

  19. Measurement of B-->K{*}(892)gamma branching fractions and CP and Isospin asymmetries.

    PubMed

    Aubert, B; Karyotakis, Y; Lees, J P; Poireau, V; Prencipe, E; Prudent, X; Tisserand, V; Garra Tico, J; Grauges, E; Martinelli, M; Palano, A; Pappagallo, M; Eigen, G; Stugu, B; Sun, L; Battaglia, M; Brown, D N; Kerth, L T; Kolomensky, Yu G; Lynch, G; Osipenkov, I L; Tackmann, K; Tanabe, T; Hawkes, C M; Soni, N; Watson, A T; Koch, H; Schroeder, T; Asgeirsson, D J; Fulsom, B G; Hearty, C; Mattison, T S; McKenna, J A; Barrett, M; Khan, A; Randle-Conde, A; Blinov, V E; Bukin, A D; Buzykaev, A R; Druzhinin, V P; Golubev, V B; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Todyshev, K Yu; Bondioli, M; Curry, S; Eschrich, I; Kirkby, D; Lankford, A J; Lund, P; Mandelkern, M; Martin, E C; Stoker, D P; Atmacan, H; Gary, J W; Liu, F; Long, O; Vitug, G M; Yasin, Z; Zhang, L; Sharma, V; Campagnari, C; Hong, T M; Kovalskyi, D; Mazur, M A; Richman, J D; Beck, T W; Eisner, A M; Heusch, C A; Kroseberg, J; Lockman, W S; Martinez, A J; Schalk, T; Schumm, B A; Seiden, A; Wang, L; Winstrom, L O; Cheng, C H; Doll, D A; Echenard, B; Fang, F; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Andreassen, R; Mancinelli, G; Meadows, B T; Mishra, K; Sokoloff, M D; Bloom, P C; Ford, W T; Gaz, A; Hirschauer, J F; Nagel, M; Nauenberg, U; Smith, J G; Wagner, S R; Ayad, R; Toki, W H; Wilson, R J; Feltresi, E; Hauke, A; Jasper, H; Karbach, T M; Merkel, J; Petzold, A; Spaan, B; Wacker, K; Kobel, M J; Nogowski, R; Schubert, K R; Schwierz, R; Volk, A; Bernard, D; Latour, E; Verderi, M; Clark, P J; Playfer, S; Watson, J E; Andreotti, M; Bettoni, D; Bozzi, C; Calabrese, R; Cecchi, A; Cibinetto, G; Fioravanti, E; Franchini, P; Luppi, E; Munerato, M; Negrini, M; Petrella, A; Piemontese, L; Santoro, V; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Pacetti, S; Patteri, P; Peruzzi, I M; Piccolo, M; Rama, M; Zallo, A; Contri, R; Guido, E; Lo Vetere, M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Tosi, S; Chaisanguanthum, K S; Morii, M; Adametz, A; Marks, J; Schenk, S; Uwer, U; Bernlochner, F U; Klose, V; Lacker, H M; Bard, D J; Dauncey, P D; Tibbetts, M; Behera, P K; Charles, M J; Mallik, U; Cochran, J; Crawley, H B; Dong, L; Eyges, V; Meyer, W T; Prell, S; Rosenberg, E I; Rubin, A E; Gao, Y Y; Gritsan, A V; Guo, Z J; Arnaud, N; Béquilleux, J; D'Orazio, A; Davier, M; Derkach, D; Firmino da Costa, J; Grosdidier, G; Le Diberder, F; Lepeltier, V; Lutz, A M; Malaescu, B; Pruvot, S; Roudeau, P; Schune, M H; Serrano, J; Sordini, V; Stocchi, A; Wormser, G; Lange, D J; Wright, D M; Bingham, I; Burke, J P; Chavez, C A; Fry, J R; Gabathuler, E; Gamet, R; Hutchcroft, D E; Payne, D J; Touramanis, C; Bevan, A J; Clarke, C K; Di Lodovico, F; Sacco, R; Sigamani, M; Cowan, G; Paramesvaran, S; Wren, A C; Brown, D N; Davis, C L; Denig, A G; Fritsch, M; Gradl, W; Hafner, A; Alwyn, K E; Bailey, D; Barlow, R J; Jackson, G; Lafferty, G D; West, T J; Yi, J I; Anderson, J; Chen, C; Jawahery, A; Roberts, D A; Simi, G; Tuggle, J M; Dallapiccola, C; Salvati, E; Saremi, S; Cowan, R; Dujmic, D; Fisher, P H; Henderson, S W; Sciolla, G; Spitznagel, M; Yamamoto, R K; Zhao, M; Patel, P M; Robertson, S H; Schram, M; Lazzaro, A; Lombardo, V; Palombo, F; Stracka, S; Bauer, J M; Cremaldi, L; Godang, R; Kroeger, R; Sonnek, P; Summers, D J; Zhao, H W; Simard, M; Taras, P; Nicholson, H; De Nardo, G; Lista, L; Monorchio, D; Onorato, G; Sciacca, C; Raven, G; Snoek, H L; Jessop, C P; Knoepfel, K J; Losecco, J M; Wang, W F; Corwin, L A; Honscheid, K; Kagan, H; Kass, R; Morris, J P; Rahimi, A M; Regensburger, J J; Sekula, S J; Wong, Q K; Blount, N L; Brau, J; Frey, R; Igonkina, O; Kolb, J A; Lu, M; Rahmat, R; Sinev, N B; Strom, D; Strube, J; Torrence, E; Castelli, G; Gagliardi, N; Margoni, M; Morandin, M; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Voci, C; Del Amo Sanchez, P; Ben-Haim, E; Bonneaud, G R; Briand, H; Chauveau, J; Hamon, O; Leruste, Ph; Marchiori, G; Ocariz, J; Perez, A; Prendki, J; Sitt, S; Gladney, L; Biasini, M; Manoni, E; Angelini, C; Batignani, G; Bettarini, S; Calderini, G; Carpinelli, M; Cervelli, A; Forti, F; Giorgi, M A; Lusiani, A; Morganti, M; Neri, N; Paoloni, E; Rizzo, G; Walsh, J J; Lopes Pegna, D; Lu, C; Olsen, J; Smith, A J S; Telnov, A V; Anulli, F; Baracchini, E; Cavoto, G; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Jackson, P D; Li Gioi, L; Mazzoni, M A; Morganti, S; Piredda, G; Renga, F; Voena, C; Ebert, M; Hartmann, T; Schröder, H; Waldi, R; Adye, T; Franek, B; Olaiya, E O; Wilson, F F; Emery, S; Esteve, L; Hamel de Monchenault, G; Kozanecki, W; Vasseur, G; Yèche, Ch; Zito, M; Allen, M T; Aston, D; Bartoldus, R; Benitez, J F; Cenci, R; Coleman, J P; Convery, M R; Dingfelder, J C; Dorfan, J; Dubois-Felsmann, G P; Dunwoodie, W; Field, R C; Franco Sevilla, M; Gabareen, A M; Graham, M T; Grenier, P; Hast, C; Innes, W R; Kaminski, J; Kelsey, M H; Kim, H; Kim, P; Kocian, M L; Leith, D W G S; Li, S; Lindquist, B; Luitz, S; Luth, V; Lynch, H L; Macfarlane, D B; Marsiske, H; Messner, R; Muller, D R; Neal, H; Nelson, S; O'Grady, C P; Ofte, I; Perl, M; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Snyder, A; Su, D; Sullivan, M K; Suzuki, K; Swain, S K; Thompson, J M; Va'vra, J; Wagner, A P; Weaver, M; West, C A; Wisniewski, W J; Wittgen, M; Wright, D H; Wulsin, H W; Yarritu, A K; Young, C C; Ziegler, V; Chen, X R; Liu, H; Park, W; Purohit, M V; White, R M; Wilson, J R; Burchat, P R; Edwards, A J; Miyashita, T S; Ahmed, S; Alam, M S; Ernst, J A; Pan, B; Saeed, M A; Zain, S B; Soffer, A; Spanier, S M; Wogsland, B J; Eckmann, R; Ritchie, J L; Ruland, A M; Schilling, C J; Schwitters, R F; Wray, B C; Drummond, B W; Izen, J M; Lou, X C; Bianchi, F; Gamba, D; Pelliccioni, M; Bomben, M; Bosisio, L; Cartaro, C; Della Ricca, G; Lanceri, L; Vitale, L; Azzolini, V; Lopez-March, N; Martinez-Vidal, F; Milanes, D A; Oyanguren, A; Albert, J; Banerjee, Sw; Bhuyan, B; Choi, H H F; Hamano, K; King, G J; Kowalewski, R; Lewczuk, M J; Nugent, I M; Roney, J M; Sobie, R J; Gershon, T J; Harrison, P F; Ilic, J; Latham, T E; Mohanty, G B; Puccio, E M T; Band, H R; Chen, X; Dasu, S; Flood, K T; Pan, Y; Prepost, R; Vuosalo, C O; Wu, S L

    2009-11-20

    We present an analysis of the decays B{0}-->K{*0}(892)gamma and B{+}-->K{*+}(892)gamma using a sample of about 383 x 10{6} BB[-over ] events collected with the BABAR detector at the PEP-II asymmetric energy B factory. We measure the branching fractions B(B{0}-->K{*0}gamma)=(4.47+/-0.10+/-0.16) x 10{-5} and B(B{+}-->K{*+}gamma)=(4.22+/-0.14+/-0.16) x 10{-5}. We constrain the direct CP asymmetry to be -0.033K{*}gamma)<0.028 and the isospin asymmetry to be 0.017

  20. Measurement of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC

    SciTech Connect

    Makii, H.; Miyatake, H.; Wakabayashi, Y.; Ishiyama, H.; Niki, K.; Okada, M.; Imai, N.; Watanabe, Y. X.; Hirayama, Y.; Jeong, S. C.; Shima, T.; Nishinaka, I.; Mitsuoka, S.; Nishio, K.; Chiba, S.

    2012-11-12

    We have measured the {gamma}-ray angular distribution of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC (Tokai Radioactive Ion Accelerator Complex) to accurately determine the E1 and E2 cross sections. In this experiment, we used high efficiency anti-Compton NaI(T1) spectrometers to detect a {gamma}-ray from the reaction with large S/N ratio, intense pulsed {alpha}-beams to discriminate true event from background events due to neutrons from {sup 13}C({alpha},n){sup 16}O reaction with a time-of-flight (TOF) method. We succeeded in removing a background events due to neutrons and clearly detected {gamma}-ray from the {sup 12}C({alpha}{gamma}){sup 16}O reaction with high statistics.

  1. Measurement of B-->K{*}(892)gamma branching fractions and CP and Isospin asymmetries.

    PubMed

    Aubert, B; Karyotakis, Y; Lees, J P; Poireau, V; Prencipe, E; Prudent, X; Tisserand, V; Garra Tico, J; Grauges, E; Martinelli, M; Palano, A; Pappagallo, M; Eigen, G; Stugu, B; Sun, L; Battaglia, M; Brown, D N; Kerth, L T; Kolomensky, Yu G; Lynch, G; Osipenkov, I L; Tackmann, K; Tanabe, T; Hawkes, C M; Soni, N; Watson, A T; Koch, H; Schroeder, T; Asgeirsson, D J; Fulsom, B G; Hearty, C; Mattison, T S; McKenna, J A; Barrett, M; Khan, A; Randle-Conde, A; Blinov, V E; Bukin, A D; Buzykaev, A R; Druzhinin, V P; Golubev, V B; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Todyshev, K Yu; Bondioli, M; Curry, S; Eschrich, I; Kirkby, D; Lankford, A J; Lund, P; Mandelkern, M; Martin, E C; Stoker, D P; Atmacan, H; Gary, J W; Liu, F; Long, O; Vitug, G M; Yasin, Z; Zhang, L; Sharma, V; Campagnari, C; Hong, T M; Kovalskyi, D; Mazur, M A; Richman, J D; Beck, T W; Eisner, A M; Heusch, C A; Kroseberg, J; Lockman, W S; Martinez, A J; Schalk, T; Schumm, B A; Seiden, A; Wang, L; Winstrom, L O; Cheng, C H; Doll, D A; Echenard, B; Fang, F; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Andreassen, R; Mancinelli, G; Meadows, B T; Mishra, K; Sokoloff, M D; Bloom, P C; Ford, W T; Gaz, A; Hirschauer, J F; Nagel, M; Nauenberg, U; Smith, J G; Wagner, S R; Ayad, R; Toki, W H; Wilson, R J; Feltresi, E; Hauke, A; Jasper, H; Karbach, T M; Merkel, J; Petzold, A; Spaan, B; Wacker, K; Kobel, M J; Nogowski, R; Schubert, K R; Schwierz, R; Volk, A; Bernard, D; Latour, E; Verderi, M; Clark, P J; Playfer, S; Watson, J E; Andreotti, M; Bettoni, D; Bozzi, C; Calabrese, R; Cecchi, A; Cibinetto, G; Fioravanti, E; Franchini, P; Luppi, E; Munerato, M; Negrini, M; Petrella, A; Piemontese, L; Santoro, V; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Pacetti, S; Patteri, P; Peruzzi, I M; Piccolo, M; Rama, M; Zallo, A; Contri, R; Guido, E; Lo Vetere, M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Tosi, S; Chaisanguanthum, K S; Morii, M; Adametz, A; Marks, J; Schenk, S; Uwer, U; Bernlochner, F U; Klose, V; Lacker, H M; Bard, D J; Dauncey, P D; Tibbetts, M; Behera, P K; Charles, M J; Mallik, U; Cochran, J; Crawley, H B; Dong, L; Eyges, V; Meyer, W T; Prell, S; Rosenberg, E I; Rubin, A E; Gao, Y Y; Gritsan, A V; Guo, Z J; Arnaud, N; Béquilleux, J; D'Orazio, A; Davier, M; Derkach, D; Firmino da Costa, J; Grosdidier, G; Le Diberder, F; Lepeltier, V; Lutz, A M; Malaescu, B; Pruvot, S; Roudeau, P; Schune, M H; Serrano, J; Sordini, V; Stocchi, A; Wormser, G; Lange, D J; Wright, D M; Bingham, I; Burke, J P; Chavez, C A; Fry, J R; Gabathuler, E; Gamet, R; Hutchcroft, D E; Payne, D J; Touramanis, C; Bevan, A J; Clarke, C K; Di Lodovico, F; Sacco, R; Sigamani, M; Cowan, G; Paramesvaran, S; Wren, A C; Brown, D N; Davis, C L; Denig, A G; Fritsch, M; Gradl, W; Hafner, A; Alwyn, K E; Bailey, D; Barlow, R J; Jackson, G; Lafferty, G D; West, T J; Yi, J I; Anderson, J; Chen, C; Jawahery, A; Roberts, D A; Simi, G; Tuggle, J M; Dallapiccola, C; Salvati, E; Saremi, S; Cowan, R; Dujmic, D; Fisher, P H; Henderson, S W; Sciolla, G; Spitznagel, M; Yamamoto, R K; Zhao, M; Patel, P M; Robertson, S H; Schram, M; Lazzaro, A; Lombardo, V; Palombo, F; Stracka, S; Bauer, J M; Cremaldi, L; Godang, R; Kroeger, R; Sonnek, P; Summers, D J; Zhao, H W; Simard, M; Taras, P; Nicholson, H; De Nardo, G; Lista, L; Monorchio, D; Onorato, G; Sciacca, C; Raven, G; Snoek, H L; Jessop, C P; Knoepfel, K J; Losecco, J M; Wang, W F; Corwin, L A; Honscheid, K; Kagan, H; Kass, R; Morris, J P; Rahimi, A M; Regensburger, J J; Sekula, S J; Wong, Q K; Blount, N L; Brau, J; Frey, R; Igonkina, O; Kolb, J A; Lu, M; Rahmat, R; Sinev, N B; Strom, D; Strube, J; Torrence, E; Castelli, G; Gagliardi, N; Margoni, M; Morandin, M; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Voci, C; Del Amo Sanchez, P; Ben-Haim, E; Bonneaud, G R; Briand, H; Chauveau, J; Hamon, O; Leruste, Ph; Marchiori, G; Ocariz, J; Perez, A; Prendki, J; Sitt, S; Gladney, L; Biasini, M; Manoni, E; Angelini, C; Batignani, G; Bettarini, S; Calderini, G; Carpinelli, M; Cervelli, A; Forti, F; Giorgi, M A; Lusiani, A; Morganti, M; Neri, N; Paoloni, E; Rizzo, G; Walsh, J J; Lopes Pegna, D; Lu, C; Olsen, J; Smith, A J S; Telnov, A V; Anulli, F; Baracchini, E; Cavoto, G; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Jackson, P D; Li Gioi, L; Mazzoni, M A; Morganti, S; Piredda, G; Renga, F; Voena, C; Ebert, M; Hartmann, T; Schröder, H; Waldi, R; Adye, T; Franek, B; Olaiya, E O; Wilson, F F; Emery, S; Esteve, L; Hamel de Monchenault, G; Kozanecki, W; Vasseur, G; Yèche, Ch; Zito, M; Allen, M T; Aston, D; Bartoldus, R; Benitez, J F; Cenci, R; Coleman, J P; Convery, M R; Dingfelder, J C; Dorfan, J; Dubois-Felsmann, G P; Dunwoodie, W; Field, R C; Franco Sevilla, M; Gabareen, A M; Graham, M T; Grenier, P; Hast, C; Innes, W R; Kaminski, J; Kelsey, M H; Kim, H; Kim, P; Kocian, M L; Leith, D W G S; Li, S; Lindquist, B; Luitz, S; Luth, V; Lynch, H L; Macfarlane, D B; Marsiske, H; Messner, R; Muller, D R; Neal, H; Nelson, S; O'Grady, C P; Ofte, I; Perl, M; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Snyder, A; Su, D; Sullivan, M K; Suzuki, K; Swain, S K; Thompson, J M; Va'vra, J; Wagner, A P; Weaver, M; West, C A; Wisniewski, W J; Wittgen, M; Wright, D H; Wulsin, H W; Yarritu, A K; Young, C C; Ziegler, V; Chen, X R; Liu, H; Park, W; Purohit, M V; White, R M; Wilson, J R; Burchat, P R; Edwards, A J; Miyashita, T S; Ahmed, S; Alam, M S; Ernst, J A; Pan, B; Saeed, M A; Zain, S B; Soffer, A; Spanier, S M; Wogsland, B J; Eckmann, R; Ritchie, J L; Ruland, A M; Schilling, C J; Schwitters, R F; Wray, B C; Drummond, B W; Izen, J M; Lou, X C; Bianchi, F; Gamba, D; Pelliccioni, M; Bomben, M; Bosisio, L; Cartaro, C; Della Ricca, G; Lanceri, L; Vitale, L; Azzolini, V; Lopez-March, N; Martinez-Vidal, F; Milanes, D A; Oyanguren, A; Albert, J; Banerjee, Sw; Bhuyan, B; Choi, H H F; Hamano, K; King, G J; Kowalewski, R; Lewczuk, M J; Nugent, I M; Roney, J M; Sobie, R J; Gershon, T J; Harrison, P F; Ilic, J; Latham, T E; Mohanty, G B; Puccio, E M T; Band, H R; Chen, X; Dasu, S; Flood, K T; Pan, Y; Prepost, R; Vuosalo, C O; Wu, S L

    2009-11-20

    We present an analysis of the decays B{0}-->K{*0}(892)gamma and B{+}-->K{*+}(892)gamma using a sample of about 383 x 10{6} BB[-over ] events collected with the BABAR detector at the PEP-II asymmetric energy B factory. We measure the branching fractions B(B{0}-->K{*0}gamma)=(4.47+/-0.10+/-0.16) x 10{-5} and B(B{+}-->K{*+}gamma)=(4.22+/-0.14+/-0.16) x 10{-5}. We constrain the direct CP asymmetry to be -0.033K{*}gamma)<0.028 and the isospin asymmetry to be 0.017

  2. Measurement of Time-Dependent CP Asymmetry in B0 --> KS pi0 gamma Decays

    SciTech Connect

    Aubert, Bernard; Bona, M.; Karyotakis, Y.; Lees, J.P.; Poireau, V.; Prencipe, E.; Prudent, X.; Tisserand, V.; Garra Tico, J.; Grauges, E.; Lopez, L.; Palano, Antimo; Pappagallo, M.; Eigen, G.; Stugu, Bjarne; Sun, L.; Abrams, G.S.; Battaglia, M.; Brown, D.N.; Cahn, Robert N.; Jacobsen, R.G.; /LBL, Berkeley /Birmingham U. /Ruhr U., Bochum /Bristol U. /British Columbia U. /Brunel U. /Novosibirsk, IYF /UC, Irvine /UCLA /UC, Riverside /UC, San Diego /UC, Santa Barbara /UC, Santa Cruz /Caltech /Cincinnati U. /Colorado U. /Colorado State U. /Dortmund U. /Dresden, Tech. U. /Ecole Polytechnique /Edinburgh U. /Ferrara U. /INFN, Ferrara /Frascati /Genoa U. /INFN, Genoa /Harvard U. /Heidelberg U. /Humboldt U., Berlin /Imperial Coll., London /Iowa U. /Iowa State U. /Johns Hopkins U. /Karlsruhe U. /Orsay, LAL /LLNL, Livermore /Liverpool U. /Queen Mary, U. of London /Royal Holloway, U. of London /Louisville U. /Manchester U. /Maryland U. /Massachusetts U., Amherst /MIT /McGill U. /Consorzio Milano Ricerche /INFN, Milan /Mississippi U. /Montreal U. /Mt. Holyoke Coll. /Napoli Seconda U. /INFN, Naples /NIKHEF, Amsterdam /Notre Dame U. /Ohio State U. /Oregon U. /Padua U. /INFN, Padua /Paris U., VI-VII /Pennsylvania U. /Perugia U. /INFN, Perugia /INFN, Pisa /Princeton U. /Banca di Roma /Frascati /Rostock U. /Rutherford /DSM, DAPNIA, Saclay /South Carolina U. /SLAC /Stanford U., Phys. Dept. /SUNY, Albany /Tennessee U. /Texas U. /Texas U., Dallas /Turin U. /INFN, Turin /Trieste U. /INFN, Trieste /Valencia U., IFIC /Victoria U. /Warwick U. /Wisconsin U., Madison

    2008-10-20

    The authors measure the time-dependent CP asymmetry in B{sup 0} {yields} K{sub S}{sup 0}{pi}{sup 0}{gamma} decays for two regions of K{sub S}{sup 0}-{pi}{sup 0} invariant mass, m(K{sub S}{sup 0}{pi}{sup 0}), using the final BABAR data set of 467 x 10{sup 6} B{bar B} pairs collected at the PEP-II e{sup +}e{sup -} collider at SLAC. They find 339 {+-} 24 B{sup 0} {yields} K*{sup 0}{gamma} candidates and measure S{sub K*{gamma}} = -0.03 {+-} 0.29 {+-} 0.03 and C{sub K*{gamma}} = -0.14 {+-} 0.16 {+-} 0.03. In the range 1.1 < m(K{sub S}{sup 0}{pi}{sup 0}) < 1.8 GeV/c{sup 2} they find 133 {+-} 20 B{sup 0} {yields} K{sub S}{sup 0}{pi}{sup 0}{gamma} candidates and measure S{sub K{sub S}{sup 0}{pi}{sup 0}{gamma}} = -0.78 {+-} 0.59 {+-} 0.09 and C{sub K{sub S}{sup 0}{pi}{sup 0}{gamma}} = -0.36 {+-} 0.33 {+-} 0.04. The uncertainties are statistical and systematic, respectively.

  3. TRYAD: a Pair of CubeSats to Measure Terrestrial Gamma-ray Flash Beams

    NASA Astrophysics Data System (ADS)

    Briggs, M. S.; Wersinger, J. M.; Fogle, M., Jr.; Biaz, S.; Jenke, P.

    2015-12-01

    The Terrestrial RaYs Analysis and Detection (TRYAD) mission is designed to measure the beam profiles and tilts of Terrestrial Gamma-ray Flashes (TGFs) using a pair of CubeSats separated by several hundred km in low Earth orbit. Until now, all TGF gamma-ray measurements have been made from single locations so that there is substantial degeneracy in modeling TGF beams. TRYAD will sample the gamma-ray beam at two locations. Additionally, for many TGFs the source location will be determined using networks of ground-based very low frequency (VLF) radio receivers. With gamma-ray measurements at two positions of known location relative to the TGF source, we will be able to test and distinguish between TGF beam models. Control of satellite separation is essential to the TRYAD mission. Separation control is achieved by using ionospheric differential drag on the two satellites.

  4. Measurement of W-gamma and Z-gamma production in pp collisions at sqrt(s) = 7 TeV

    SciTech Connect

    Chatrchyan, Serguei; et al.

    2011-07-01

    A measurement of W-gamma and Z-gamma production in proton-proton collisions at sqrt(s) = 7 TeV is presented. Results are based on a data sample recorded by the CMS experiment at the LHC, corresponding to an integrated luminosity of 36 inverse picobarns. The electron and muon decay channels of the W and Z are used. The total cross sections are measured for photon transverse energy >10 GeV and spatial separation from charged leptons in the plane of pseudorapidity and azimuthal angle >0.7, and with an additional dilepton invariant mass requirement of > 50 GeV for the Z-gamma process. The following cross section times branching fraction values are found: sigma(pp to W-gamma+X) B(W to lepton neutrino) = 56.3 +/- 5.0 (stat.) +/- 5.0 (syst.) +/- 2.3 (lumi.) pb and sigma(pp to Z-gamma+X) B}(Z to lepton lepton) = 9.4 +/- 1.0 (stat.) +/- 0.6 (syst.) +/- 0.4 (lumi.) pb. These measurements are in agreement with standard model predictions. The first limits on anomalous WW gamma, ZZ gamma, and Z gamma gamma trilinear gauge couplings at sqrt(s) = 7 TeV are set

  5. Measurements of background gamma radiation on Spacelab 2

    NASA Technical Reports Server (NTRS)

    Fishman, G. J.; Paciesas, W. S.; Gregory, J. C.

    1987-01-01

    A nuclear radiation monitor (NRM) which was flown as part of the verification instrumentation on the Spacelab 2 mission (July 29 - August 6, 1985) recorded spectra every 20 seconds and counting rates in coarse energy bands on finer time scales. The gamma radiation environment on Spacelab is characterized by cosmic-ray and trapped proton secondary radiation in the Spacelab/Shuttle, earth albedo radiation, and delayed induced radioactivity in the detector and surrounding materials. It is found that passages through South Atlantic Anomaly protons produce a well-defined background enhancement.

  6. Assembly of an alpha-gamma coincidence measuring device for checking alpha decay schemes.

    PubMed

    Martín Sánchez, A; Caro Marroyo, B

    2012-09-01

    Two new chambers for measuring alpha-particle emissions have been made: a low-geometry chamber with a powerful magnet to eliminate conversion electrons, and an alpha-gamma coincidence chamber. Both devices incorporate a high-resolution Si detector, and the second chamber, a low-energy Ge detector as well. A dual parameter multichannel analyzer was used to register coincidences in the second device. Alpha-particle and gamma-ray detectors work simultaneously in both individual and dual modes, providing single and coincidence spectra. Some preliminary alpha-gamma coincidence spectra have been obtained.

  7. A system for the measurement of delayed neutrons and gammas from special nuclear materials

    DOE PAGES

    Andrews, M. T.; Corcoran, E. C.; Goorley, J. T.; Kelly, D. G.

    2014-11-27

    The delayed neutron counting (DNC) system at the Royal Military College of Canada has been upgraded to accommodate concurrent delayed neutron and gamma measurements. This delayed neutron and gamma counting (DNGC) system uses a SLOWPOKE-2 reactor to irradiate fissile materials before their transfer to a counting arrangement consisting of six ³He and one HPGe detector. The application of this system is demonstrated in an example where delayed neutron and gamma emissions are used in complement to examine ²³³U content and determine fissile mass with an average relative error and accuracy of -2.2 and 1.5 %, respectively.

  8. A system for the measurement of delayed neutrons and gammas from special nuclear materials

    SciTech Connect

    Andrews, M. T.; Corcoran, E. C.; Goorley, J. T.; Kelly, D. G.

    2015-03-01

    The delayed neutron counting (DNC) system at the Royal Military College of Canada has been upgraded to accommodate concurrent delayed neutron and gamma measurements. This delayed neutron and gamma counting (DNGC) system uses a SLOWPOKE-2 reactor to irradiate fissile materials before their transfer to a counting arrangement consisting of six ³He and one HPGe detector. The application of this system is demonstrated in an example where delayed neutron and gamma emissions are used in complement to examine ²³³U content and determine fissile mass with an average relative error and accuracy of -2.2 and 1.5 %, respectively.

  9. Rapid In-Situ Measurement of Gamma Activity in Soil for Environmental Assessment

    NASA Astrophysics Data System (ADS)

    Honeycutt, T. K.

    2003-12-01

    In-situ measurements of gamma radiation in soil are used as a rapid, low-cost, non-intrusive alternative to conventional sampling and analysis methods in the preliminary assessment of environmental impacts to watersheds at the Savannah River Site (SRS). The method resolves the ambient gamma-radiation field near ground surface into background and residual components and provides radionuclide-specific soil activity determination. The efficacy of the method has been evaluated and compares favorably with conventional gamma-PHA soil analyses and aerial survey data. The method has garnered regulatory approval and is being successfully deployed to evaluate the impact of Cs-137 contamination from CERCLA sites.

  10. Measuring planetary neutron albedo fluxes by remote gamma-ray sensing

    NASA Technical Reports Server (NTRS)

    Haines, E. L.; Metzger, A. E.

    1984-01-01

    In order to measure the planetary neutron albedo fluxes, a neutron-absorbing shield which emits gamma rays of characteristic energy and serves as a neutron detector, is added to a gamma-ray spectrometer (GRS). The gamma rays representing the neutron flux are observed against interference consisting of cosmic gamma rays, planetary continuum and line emission, and gamma rays arising from the interaction of cosmic rays with the GRS and the spacecraft. The uncertainty and minimum detection limits in neutron albedo fluxes are calculated for two missions, a lunar orbiter and a comet nucleus rendezvous. A GRS on a lunar orbiter at 100 km altitude detects a thermal neutron albedo flux as low as 0.002/sq cm/s and an expected flux of about 0.6/sq cm/s is measured with an uncertainty of 0.001/sq cm/s, for a 100 h observation period. For the comet nucleus, again in a 100 h observing period, a thermal neutron albedo flux is detected at a level of 0.006/sq cm/s and an expected flux of about 0.4/sq cm/s is measured with an uncertainty of 0.004/sq cm/s. The expanded geological capabilities made possible by this technique include improvements in H sensitivity, spatial resolution, and measurement depth; and an improved model of induced gamma-ray emission.

  11. Environmental gamma dosimetry with OSL of alpha-Al(2)O(3):C for in situ sediment measurements.

    PubMed

    Richter, D; Dombrowski, H; Neumaier, S; Guibert, P; Zink, A C

    2010-09-01

    The physical properties of alpha-Al(2)O(3):C are very similar to that of quartz, which make it an attractive dosimetric material for geological and archaeological dating applications. Storage experiments in an ultra-low-radiation underground environment (UDO at PTB) and gamma-ray spectrometry show that the optically stimulated luminescence (OSL) signal of this material does neither suffer from a significant inherent background caused by traces of radionuclides (<6 microGy a(-1)) nor from fading. After having performed a simple calibration procedure, gamma dosimetry based on alpha-Al(2)O(3):C detectors, which were exposed in a brick block and a lead castle for different periods of time, provided concordant results with dose values derived from independent gamma-ray spectrometric measurements using high-purity germanium and NaI:Tl detectors. These investigations indirectly confirm both the absence of a significant inherent background and fading of the detector material. Small doses of a few micro gray accumulated in short exposure times to environmental radiation can be accurately measured, even when doses (i.e. transport dose) much larger than the actual environmental dose have to be subtracted. It is shown that the OSL signal caused by small transport doses can be easily and reproducibly reset even under difficult field conditions by illuminating the dosemeters with the blue light from Luxeon LEDs. Summarised, alpha-Al(2)O(3):C appears to be the material of choice for dosimetric dating applications of quartz or related materials, when analysed by using OSL. PMID:20534630

  12. Time-integrated measurements of $\\gamma$ at the Tevatron and prospects

    SciTech Connect

    Squillacioti, Paola

    2010-12-01

    The measurement of CP-violating asymmetries and branching ratios of B {yields} DK modes allows a theoretically-clean extraction of the CKM angle {gamma}. We report recent CDF measurements with Cabibbo suppressed ({pi}{pi}, KK) or doubly Cabibbo suppressed (K{sup +}{pi}{sup -}) D decays. These measurements are performed for the first time in hadron collisions.

  13. Electroweak physics: measurement of w gamma and z gamma production in pp-bar collisions at s**(1/2) = 1.96 tev

    SciTech Connect

    Acosta, D.; The CDF Collaboration

    2005-02-02

    The Standard Model predictions for W{gamma} and Z{gamma} production are tested using an integrated luminosity of 200 pb{sup -1} of p{bar p} collision data collected at the Collider Detector at Fermilab. The cross sections are measured by selecting leptonic decays of the W and Z bosons, and photons with transverse energy E{sub T} > 7 GeV that are well separated from leptons. The production cross sections and kinematic distributions for the W{gamma} and Z{gamma} data are compared to SM predictions.

  14. Measurement of Branching Fractions and Mass Spectra of B to K pi pi gamma

    SciTech Connect

    Aubert, B.; Barate, R.; Boutigny, D.; Couderc, F.; Karyotakis, Y.; Lees, J.P.; Poireau, V.; Tisserand, V.; Zghiche, A.; Grauges, E.; Palano, A.; Pappagallo, M.; Pompili, A.; Chen, J.C.; Qi, N.D.; Rong, G.; Wang, P.; Zhu, Y.S.; Eigen, G.; Ofte, I.; Stugu, B. /Bergen U. /LBL, Berkeley /UC, Berkeley /Birmingham U. /Ruhr U., Bochum /Bristol U. /British Columbia U. /Brunel U. /Novosibirsk, IYF /UC, Irvine /UCLA /UC, Riverside /UC, San Diego /UC, Santa Barbara /UC, Santa Cruz /Caltech /Cincinnati U. /Colorado U. /Colorado State U. /Dortmund U. /Dresden, Tech. U. /Ecole Polytechnique /Edinburgh U. /Ferrara U. /INFN, Ferrara /Frascati /Genoa U. /INFN, Genoa /Harvard U. /Heidelberg U. /Imperial Coll., London /Iowa U. /Iowa State U. /Orsay, LAL /LLNL, Livermore /Liverpool U. /Queen Mary, U. of London /Royal Holloway, U. of London /Louisville U. /Manchester U. /Maryland U. /Massachusetts U., Amherst /MIT, LNS /McGill U. /Milan U. /INFN, Milan /Mississippi U. /Montreal U. /Mt. Holyoke Coll. /Naples U. /INFN, Naples /NIKHEF, Amsterdam /Notre Dame U. /Ohio State U. /Oregon U. /INFN, Padua /Padua U. /Paris U., VI-VII /Pennsylvania U. /Perugia U. /INFN, Perugia /Pisa U. /Pisa, Scuola Normale Superiore /INFN, Pisa /Prairie View A-M /Princeton U. /Rome U. /INFN, Rome /Rostock U. /Rutherford /DAPNIA, Saclay /South Carolina U. /SLAC /Stanford U., Phys. Dept. /SUNY, Albany /Tennessee U. /Texas U. /Texas U., Dallas /Turin U. /INFN, Turin /Trieste U. /INFN, Trieste /Valencia U., IFIC /Vanderbilt U. /Victoria U. /Warwick U. /Wisconsin U., Madison /Yale U.

    2005-07-12

    The authors present a measurement of the partial branching fractions and mass spectra of the exclusive radiative penguin processes B {yields} K{pi}{pi}{gamma} in the range m{sub K{pi}{pi}} < 1.8 GeV/c{sup 2}. They reconstruct four final states: K{sup +}{pi}{sup -}{pi}{sup +}{gamma}, K{sup +}{pi}{sup -}{pi}{sup 0}{gamma}, K{sub S}{sup 0}{pi}{sup -}{pi}{sup +}{gamma}, and K{sub S}{sup 0}{pi}{sup +}{pi}{sup 0}{gamma}, where K{sub S}{sup 0} {yields} {pi}{sup +}{pi}{sup -}. Using 232 million e{sup +}e{sup -} {yields} B{bar B} events recorded by the BABAR experiment at the PEP-II asymmetric-energy storage ring, they measure the branching fractions {Beta}(B{sup +} {yields} K{sup +}{pi}{sup -}{pi}{sup +}{gamma}) = (2.95 {+-} 0.13(stat.) {+-} 0.20(syst)) x 10{sup -5}, {Beta}(B{sup 0} {yields} K{sup +}{pi}{sup -}{pi}{sup 0}{gamma}) = (4.07 {+-} 0.22(stat.) {+-} 0.31(syst.)) x 10{sup -5}, {Beta}(B{sup 0} {yields} K{sup 0}{pi}{sup +}{pi}{sup -}{gamma}) = (1.85 {+-} 0.21(stat.) {+-} 0.12(syst.)) x 10{sup -5}, and {Beta}(B{sup +} {yields} K{sup 0}{pi}{sup +}{pi}{sup 0}{gamma}) = (4.56 {+-} 0.42(stat.) {+-} 0.31(syst.)) x 10{sup -5}.

  15. Unfolding the fission prompt gamma-ray energy and multiplicity distribution measured by DANCE

    SciTech Connect

    Chyzh, A; Wu, C Y; Bredeweg, T; Couture, A; Jandel, M; Ullmann, J; Laptev, A

    2010-10-16

    The nearly energy independence of the {gamma}-ray efficiency and multiplicity response for the DANCE array, the unusual characteristic elucidated in our early technical report (LLNL-TR-452298), gives one a unique opportunity to derive the true prompt {gamma}-ray energy and multiplicity distribution in fission from the measurement. This unfolding procedure for the experimental data will be described in details and examples will be given to demonstrate the feasibility of reconstruction of the true distribution.

  16. Airborne time-series measurement of soil moisture using terrestrial gamma radiation

    NASA Technical Reports Server (NTRS)

    Carroll, Thomas R.; Lipinski, Daniel M.; Peck, Eugene L.

    1988-01-01

    Terrestrial gamma radiation data and independent ground-based core soil moisture data are analyzed. They reveal the possibility of using natural terrestrial gamma radiation collected from a low-flying aircraft to make reliable real-time soil moisture measurements for the upper 20 cm of soil. The airborne data were compared to the crude ground-based soil moisture data set collected at the core sites.

  17. COMBINED GAMMA-RAY AND NEUTRON DETECTOR FOR MEASURING THE CHEMICAL COMPOSITION OF AIRLESS PLANETARY BODIES.

    SciTech Connect

    Lawrence, David J. ,; Barraclough, B. L.; Feldman, W. C.; Prettyman, T. H.; Wiens, R. C.

    2001-01-01

    Galactic cosmic rays (GCR) constant1,y itnpinge all planetary bodies and produce characteristic gamma-ray lines and leakage neutrons as reaction products. Together with gamma-ray lines produced by radioactive decay, these nuclear emissions provide a powerful technique for remotely measuring the chemical composition of airless planetary surfaces. While lunar gamma-ray spectroscopy was first demonstrated with Apollo Gamma-Ray measurements, the full value of combined gamma-ray and neutron spectroscopy was shown for the first time with the Lunar Prospector Gamma-Ray (LP-GRS) and Neutron Spectrometers (LP-NS). Any new planetary mission will likely have the requirement that instrument mass and power be kept to a minimum. To satisfy such requirements, we have been designing a GR/NS instrument which combines all the functionality of the LP-GRS and LP-NS for a fraction of the mass and power. Specifically, our design uses a BGO scintillator crystal to measure gamma-rays from 0.5-10 MeV. A borated plastic scintillator and a lithium gliiss scintillator are used to separately measure thermal, epithermal, and fast neutrons as well as serve as an anticoincidence shield for the BGO. All three scintillators are packaged together in a compact phoswich design. Modifications to this design could include a CdZnTe gamma-ray detector for enhanced energy resolution at low energies (0.5-3 MeV). While care needs to be taken to ensure that an adequate count rate is achieved for specific mission designs, previous mission successes demonstrate that a cornbined GR/NS provides essential information about planetary surfaces.

  18. Proposed experiment to measure {gamma}-rays from the thermal neutron capture of gadolinium

    SciTech Connect

    Yano, Takatomi; Ou, I.; Izumi, T.; Yamaguchi, R.; Mori, T.; Sakuda, M.

    2012-11-12

    Gadolinium-157 ({sup 157}Gd) has the largest thermal neutron capture cross section among any stable nuclei. The thermal neutron capture yields {gamma}-ray cascade with total energy of about 8 MeV. Because of these characteristics, Gd is applied for the recent neutrino detectors. Here, we propose an experiment to measure the multiplicity and the angular correlation of {gamma}-rays from the Gd neutron capture. With these information, we expect the improved identification of the Gd neutron capture.

  19. [Welding arc temperature field measurements based on Boltzmann spectrometry].

    PubMed

    Si, Hong; Hua, Xue-Ming; Zhang, Wang; Li, Fang; Xiao, Xiao

    2012-09-01

    Arc plasma, as non-uniform plasma, has complicated energy and mass transport processes in its internal, so plasma temperature measurement is of great significance. Compared with absolute spectral line intensity method and standard temperature method, Boltzmann plot measuring is more accurate and convenient. Based on the Boltzmann theory, the present paper calculates the temperature distribution of the plasma and analyzes the principle of lines selection by real time scanning the space of the TIG are measurements. PMID:23240385

  20. Extended use of alanine irradiated in experimental reactor for combined gamma- and neutron-dose assessment by ESR spectroscopy and thermal neutron fluence assessment by measurement of (14)C by LSC.

    PubMed

    Bartoníček, B; Kučera, J; Světlík, I; Viererbl, L; Lahodová, Z; Tomášková, L; Cabalka, M

    2014-11-01

    Gamma- and neutron doses in an experimental reactor were measured using alanine/electron spin resonance (ESR) spectrometry. The absorbed dose in alanine was decomposed into contributions caused by gamma and neutron radiation using neutron kerma factors. To overcome a low sensitivity of the alanine/ESR response to thermal neutrons, a novel method has been proposed for the assessment of a thermal neutron flux using the (14)N(n,p) (14)C reaction on nitrogen present in alanine and subsequent measurement of (14)C by liquid scintillation counting (LSC).

  1. Nuclear data production, calculation and measurement: a global overview of the gamma heating issue

    NASA Astrophysics Data System (ADS)

    Colombier, A.-C.; Amharrak, H.; Fourmentel, D.; Ravaux, S.; Régnier, D.; Gueton, O.; Hudelot, J.-P.; Lemaire, M.

    2013-03-01

    The gamma heating evaluation in different materials found in current and future generations of nuclear reactor (EPRTM, GENIV, MTR-JHR), is becoming an important issue especially for the design of many devices (control rod, heavy reflector, in-core & out-core experiments…). This paper deals with the works started since 2009 in the Reactor Studies Department of CEA Cadarache in ordre to answer to several problematic which have been identified as well for nuclear data production and calculation as for experimental measurement methods. The selected subjects are: Development of a Monte Carlo code (FIFRELIN) to simulate the prompt fission gamma emission which represents the major part of the gamma heating production inside the core Production and qualification of new evaluations of nuclear data especially for radiative capture and inelastic neutron scattering which are the main sources of gamma heating out-core Development and qualification of a recommended method for the total gamma heating calculation using the Monte Carlo simulation code TRIPOLI-4 Development, test and qualification of new devices dedicated to the in-core gamma heating measurement as well in MTR-JHR as in zero power facilities (EOLE-MINERVE) of CEA, Cadarache to increase the experimental measurement accuracy.

  2. Measurement of Cross-sections of Yttrium (n,xn) Threshold Reactions by Means of Gamma Spectroscopy

    NASA Astrophysics Data System (ADS)

    Chudoba, P.; Kilim, S.; Wagner, V.; Vrzalova, J.; Svoboda, O.; Majerle, M.; Stefanik, M.; Suchopar, M.; Kugler, A.; Bielewicz, M.; Strugalska-Gola, E.; Szuta, M.; Hervas, D.; Herman, T.; Geier, B.

    Neutron activation and gamma spectrometry are usable also for the determination of cross-sections of different neutron reactions. We have studied the cross-section of yttrium (n,xn) threshold reactions using quasi mono-energetic neutron source based on the reaction on 7Li target at Nuclear Physics Institute of ASCR in Rez. Yttrium (n,xn) threshold reactions are suitable candidates for fast neutron field measurement by activation detectors. Fast neutron field monitoring is necessary already today at a wide range of accelerator facilities and will gain on importance in future fast reactors of generation IV, accelerator transmutation systems or fusion reactors. The knowledge of the cross-sections is crucial for such purpose. Unfortunately, the cross-section is sufficiently known only for 89Y(n,2n)88Y reaction. For higher orders of reactions there are almost no experimental data. Special attention was paid to the 89Y(n,3n)87Y reaction. The nuclei are produced, both in the ground state with half-life 79.8 hours and in the isomeric state with half-life 13.38 hours. The isomer decays mainly through the gamma transition to the ground state, the beta decay of the excited state is negligible within our accuracy. The cross-sections of both 87Y productions were analyzed.

  3. Gamma-ray spectrometry method used for radioactive waste drums characterization for final disposal at National Repository for Low and Intermediate Radioactive Waste--Baita, Romania.

    PubMed

    Done, L; Tugulan, L C; Dragolici, F; Alexandru, C

    2014-05-01

    The Radioactive Waste Management Department from IFIN-HH, Bucharest, performs the conditioning of the institutional radioactive waste in concrete matrix, in 200 l drums with concrete shield, for final disposal at DNDR - Baita, Bihor county, in an old exhausted uranium mine. This paper presents a gamma-ray spectrometry method for the characterization of the radioactive waste drums' radionuclides content, for final disposal. In order to study the accuracy of the method, a similar concrete matrix with Portland cement in a 200 l drum was used.

  4. FFTF reactor-characterization program: gamma-ray measurements and shield characterization

    SciTech Connect

    Bunch, W.L.; Moore, F.S. Jr.

    1983-02-01

    A series of experiments is to be made during the acceptance test program of the Fast Flux Test Facility (FFTF) to measure the gamma ray characteristics of the Fast Test Reactor (FTR) and to establish the performance characteristics of the reactor shield. These measurements are a part of the FFTF Reactor Characterization Program (RCP). Detailed plans have been developed for these experiments. During the initial phase of the Characteristics Program, which will be carried out in the In-Reactor Thimble (IRT), both active and passive measurement methods will be employed to obtain as much information concerning the gamma ray environment as is practical. More limited active gamma ray measurements also will be made in the Vibration Open Test Assembly (VOTA).

  5. Measurement of the branching fraction and photon energy moments of B-->Xs gamma and A(CP)(B --> X(s+d gamma)).

    PubMed

    Aubert, B; Barate, R; Bona, M; Boutigny, D; Couderc, F; Karyotakis, Y; Lees, J P; Poireau, V; Tisserand, V; Zghiche, A; Grauges, E; Palano, A; Chen, J C; Qi, N D; Rong, G; Wang, P; Zhu, Y S; Eigen, G; Ofte, I; Stugu, B; Abrams, G S; Battaglia, M; Brown, D N; Button-Shafer, J; Cahn, R N; Charles, E; Gill, M S; Groysman, Y; Jacobsen, R G; Kadyk, J A; Kerth, L T; Kolomensky, Yu G; Kukartsev, G; Lynch, G; Mir, L M; Oddone, P J; Orimoto, T J; Pripstein, M; Roe, N A; Ronan, M T; Wenzel, W A; del Amo Sanchez, P; Barrett, M; Ford, K E; Harrison, T J; Hart, A J; Hawkes, C M; Morgan, S E; Watson, A T; Goetzen, K; Held, T; Koch, H; Lewandowski, B; Pelizaeus, M; Peters, K; Schroeder, T; Steinke, M; Boyd, J T; Burke, J P; Cottingham, W N; Walker, D; Cuhadar-Donszelmann, T; Fulsom, B G; Hearty, C; Knecht, N S; Mattison, T S; McKenna, J A; Khan, A; Kyberd, P; Saleem, M; Sherwood, D J; Teodorescu, L; Blinov, V E; Bukin, A D; Druzhinin, V P; Golubev, V B; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Todyshev, K Yu; Best, D S; Bondioli, M; Bruinsma, M; Chao, M; Curry, S; Eschrich, I; Kirkby, D; Lankford, A J; Lund, P; Mandelkern, M; Mommsen, R K; Roethel, W; Stoker, D P; Abachi, S; Buchanan, C; Foulkes, S D; Gary, J W; Long, O; Shen, B C; Wang, K; Zhang, L; Hadavand, H K; Hill, E J; Paar, H P; Rahatlou, S; Sharma, V; Berryhill, J W; Campagnari, C; Cunha, A; Dahmes, B; Hong, T M; Kovalskyi, D; Richman, J D; Beck, T W; Eisner, A M; Flacco, C J; Heusch, C A; Kroseberg, J; Lockman, W S; Nesom, G; Schalk, T; Schmitz, R E; Schumm, B A; Seiden, A; Spradlin, P; Williams, D C; Wilson, M G; Albert, J; Chen, E; Dvoretskii, A; Fang, F; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Ryd, A; Samuel, A; Mancinelli, G; Meadows, B T; Sokoloff, M D; Blanc, F; Bloom, P C; Chen, S; Ford, W T; Hirschauer, J F; Kreisel, A; Nauenberg, U; Olivas, A; Ruddick, W O; Smith, J G; Ulmer, K A; Wagner, S R; Zhang, J; Chen, A; Eckhart, E A; Soffer, A; Toki, W H; Wilson, R J; Winklmeier, F; Zeng, Q; Altenburg, D D; Feltresi, E; Hauke, A; Jasper, H; Petzold, A; Spaan, B; Brandt, T; Klose, V; Lacker, H M; Mader, W F; Nogowski, R; Schubert, J; Schubert, K R; Schwierz, R; Sundermann, J E; Volk, A; Bernard, D; Bonneaud, G R; Grenier, P; Latour, E; Thiebaux, Ch; Verderi, M; Bard, D J; Clark, P J; Gradl, W; Muheim, F; Playfer, S; Robertson, A I; Xie, Y; Andreotti, M; Bettoni, D; Bozzi, C; Calabrese, R; Cibinetto, G; Luppi, E; Negrini, M; Petrella, A; Piemontese, L; Prencipe, E; Anulli, F; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Pacetti, S; Patteri, P; Peruzzi, I M; Piccolo, M; Rama, M; Zallo, A; Buzzo, A; Capra, R; Contri, R; Lo Vetere, M; Macri, M M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Santroni, A; Tosi, S; Brandenburg, G; Chaisanguanthum, K S; Morii, M; Wu, J; Dubitzky, R S; Marks, J; Schenk, S; Uwer, U; Bhimji, W; Bowerman, D A; Dauncey, P D; Egede, U; Flack, R L; Nash, J A; Nikolich, M B; Panduro Vazquez, W; Chai, X; Charles, M J; Mallik, U; Meyer, N T; Ziegler, V; Cochran, J; Crawley, H B; Dong, L; Eyges, V; Meyer, W T; Prell, S; Rosenberg, E I; Rubin, A E; Gritsan, A V; Fritsch, M; Schott, G; Arnaud, N; Davier, M; Grosdidier, G; Höcker, A; Le Diberder, F; Lepeltier, V; Lutz, A M; Oyanguren, A; Pruvot, S; Rodier, S; Roudeau, P; Schune, M H; Stocchi, A; Wang, W F; Wormser, G; Cheng, C H; Lange, D J; Wright, D M; Chavez, C A; Forster, I J; Fry, J R; Gabathuler, E; Gamet, R; George, K A; Hutchcroft, D E; Payne, D J; Schofield, K C; Touramanis, C; Bevan, A J; Di Lodovico, F; Menges, W; Sacco, R; Cowan, G; Flaecher, H U; Hopkins, D A; Jackson, P S; McMahon, T R; Ricciardi, S; Salvatore, F; Wren, A C; Brown, D N; Davis, C L; Allison, J; Barlow, N R; Barlow, R J; Chia, Y M; Edgar, C L; Lafferty, G D; Naisbit, M T; Williams, J C; Yi, J I; Chen, C; Hulsbergen, W D; Jawahery, A; Lae, C K; Roberts, D A; Simi, G; Blaylock, G; Dallapiccola, C; Hertzbach, S S; Li, X; Moore, T B; Saremi, S; Staengle, H; Cowan, R; Sciolla, G; Sekula, S J; Spitznagel, M; Taylor, F; Yamamoto, R K; Kim, H; Patel, P M; Robertson, S H; Lazzaro, A; Lombardo, V; Palombo, F; Bauer, J M; Cremaldi, L; Eschenburg, V; Godang, R; Kroeger, R; Sanders, D A; Summers, D J; Zhao, H W; Brunet, S; Côté, D; Taras, P; Viaud, F B; Nicholson, H; Cavallo, N; De Nardo, G; Fabozzi, F; Gatto, C; Lista, L; Monorchio, D; Paolucci, P; Piccolo, D; Sciacca, C; Baak, M; Raven, G; Snoek, H L; Jessop, C P; LoSecco, J M; Allmendinger, T; Benelli, G; Gan, K K; Honscheid, K; Hufnagel, D; Jackson, P D; Kagan, H; Kass, R; Rahimi, A M; Ter-Antonyan, R; Wong, Q K; Blount, N L; Brau, J; Frey, R; Igonkina, O; Lu, M; Potter, C T; Rahmat, R; Sinev, N B; Strom, D; Strube, J; Torrence, E; Galeazzi, F; Gaz, A; Margoni, M; Morandin, M; Pompili, A; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Voci, C; Benayoun, M; Chauveau, J; David, P; Del Buono, L; de la Vaissière, Ch; Hamon, O; Hartfiel, B L; John, M J J; Malclès, J; Ocariz, J; Roos, L; Therin, G; Behera, P K; Gladney, L; Panetta, J; Biasini, M; Covarelli, R; Angelini, C; Batignani, G; Bettarini, S; Bucci, F; Calderini, G; Carpinelli, M; Cenci, R; Forti, F; Giorgi, M A; Lusiani, A; Marchiori, G; Mazur, M A; Morganti, M; Neri, N; Paoloni, E; Rizzo, G; Walsh, J J; Haire, M; Judd, D; Wagoner, D E; Biesiada, J; Danielson, N; Elmer, P; Lau, Y P; Lu, C; Olsen, J; Smith, A J S; Telnov, A V; Bellini, F; Cavoto, G; D'Orazio, A; del Re, D; Di Marco, E; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Li Gioi, L; Mazzoni, M A; Morganti, S; Piredda, G; Polci, F; Safai Tehrani, F; Voena, C; Ebert, M; Schröder, H; Waldi, R; Adye, T; De Groot, N; Franek, B; Olaiya, E O; Wilson, F F; Aleksan, R; Emery, S; Gaidot, A; Ganzhur, S F; Hamel de Monchenault, G; Kozanecki, W; Legendre, M; Vasseur, G; Yèche, Ch; Zito, M; Chen, X R; Liu, H; Park, W; Purohit, M V; Wilson, J R; Allen, M T; Aston, D; Bartoldus, R; Bechtle, P; Berger, N; Claus, R; Coleman, J P; Convery, M R; Cristinziani, M; Dingfelder, J C; Dorfan, J; Dubois-Felsmann, G P; Dujmic, D; Dunwoodie, W; Field, R C; Glanzman, T; Gowdy, S J; Graham, M T; Halyo, V; Hast, C; Hryn'ova, T; Innes, W R; Kelsey, M H; Kim, P; Leith, D W G S; Li, S; Libby, J; Luitz, S; Luth, V; Lynch, H L; MacFarlane, D B; Marsiske, H; Messner, R; Muller, D R; O'Grady, C P; Ozcan, V E; Perazzo, A; Perl, M; Pulliam, T; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Snyder, A; Stelzer, J; Su, D; Sullivan, M K; Suzuki, K; Swain, S K; Thompson, J M; Tinslay, J S; Va'vra, J; van Bakel, N; Weaver, M; Weinstein, A J R; Wisniewski, W J; Wittgen, M; Wright, D H; Yarritu, A K; Yi, K; Young, C C; Burchat, P R; Edwards, A J; Majewski, S A; Petersen, B A; Roat, C; Wilden, L; Ahmed, S; Alam, M S; Bula, R; Ernst, J A; Jain, V; Pan, B; Saeed, M A; Wappler, F R; Zain, S B; Bugg, W; Krishnamurthy, M; Spanier, S M; Eckmann, R; Ritchie, J L; Satpathy, A; Schilling, C J; Schwitters, R F; Izen, J M; Lou, X C; Ye, S; Bianchi, F; Gallo, F; Gamba, D; Bomben, M; Bosisio, L; Cartaro, C; Cossutti, F; Della Ricca, G; Dittongo, S; Lanceri, L; Vitale, L; Azzolini, V; Martinez-Vidal, F; Banerjee, Sw; Bhuyan, B; Brown, C M; Fortin, D; Hamano, K; Kowalewski, R; Nugent, I M; Roney, J M; Sobie, R J; Back, J J; Harrison, P F; Latham, T E; Mohanty, G B; Pappagallo, M; Band, H R; Chen, X; Cheng, B; Dasu, S; Datta, M; Flood, K T; Hollar, J J; Kutter, P E; Mellado, B; Mihalyi, A; Pan, Y; Pierini, M; Prepost, R; Wu, S L; Yu, Z; Neal, H

    2006-10-27

    The photon spectrum in B-->Xs gamma decay, where Xs is any strange hadronic state, is studied using a data sample of 88.5 x 10(6) e+ e- --> Upsilon(4S) --> BB decays collected by the BABAR experiment at the Stanford Linear Accelerator Center. The partial branching fraction, DeltaB(B --> Xs gamma) = (3.67+/-0.29(stat)+/-0.34(syst)+/-0.29(model)) x 10(-4), the first moment gamma> = 2.288+/-0.025+/-0.017+/-0.015 GeV, and the second moment E2(gamma) = 0.0328+/-0.0040+/-0.0023+/-0.0036 GeV2 are measured for the photon energy range 1.9 GeV < E gamma < 2.7 GeV. They are also measured for narrower E gamma ranges. The moments are then fit to recent theoretical calculations to extract the heavy quark expansion parameters m(b) and mu2(pi) and to extrapolate the partial branching fraction to E gamma > 1.6 GeV. In addition, the direct CP asymmetry A(CP)(B-->X(s+d gamma) is measured to be -0.110+/-0.115(stat)+/-0.017(syst). PMID:17155462

  6. Measurement of the branching fraction and photon energy moments of B-->Xs gamma and A(CP)(B --> X(s+d gamma)).

    PubMed

    Aubert, B; Barate, R; Bona, M; Boutigny, D; Couderc, F; Karyotakis, Y; Lees, J P; Poireau, V; Tisserand, V; Zghiche, A; Grauges, E; Palano, A; Chen, J C; Qi, N D; Rong, G; Wang, P; Zhu, Y S; Eigen, G; Ofte, I; Stugu, B; Abrams, G S; Battaglia, M; Brown, D N; Button-Shafer, J; Cahn, R N; Charles, E; Gill, M S; Groysman, Y; Jacobsen, R G; Kadyk, J A; Kerth, L T; Kolomensky, Yu G; Kukartsev, G; Lynch, G; Mir, L M; Oddone, P J; Orimoto, T J; Pripstein, M; Roe, N A; Ronan, M T; Wenzel, W A; del Amo Sanchez, P; Barrett, M; Ford, K E; Harrison, T J; Hart, A J; Hawkes, C M; Morgan, S E; Watson, A T; Goetzen, K; Held, T; Koch, H; Lewandowski, B; Pelizaeus, M; Peters, K; Schroeder, T; Steinke, M; Boyd, J T; Burke, J P; Cottingham, W N; Walker, D; Cuhadar-Donszelmann, T; Fulsom, B G; Hearty, C; Knecht, N S; Mattison, T S; McKenna, J A; Khan, A; Kyberd, P; Saleem, M; Sherwood, D J; Teodorescu, L; Blinov, V E; Bukin, A D; Druzhinin, V P; Golubev, V B; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Todyshev, K Yu; Best, D S; Bondioli, M; Bruinsma, M; Chao, M; Curry, S; Eschrich, I; Kirkby, D; Lankford, A J; Lund, P; Mandelkern, M; Mommsen, R K; Roethel, W; Stoker, D P; Abachi, S; Buchanan, C; Foulkes, S D; Gary, J W; Long, O; Shen, B C; Wang, K; Zhang, L; Hadavand, H K; Hill, E J; Paar, H P; Rahatlou, S; Sharma, V; Berryhill, J W; Campagnari, C; Cunha, A; Dahmes, B; Hong, T M; Kovalskyi, D; Richman, J D; Beck, T W; Eisner, A M; Flacco, C J; Heusch, C A; Kroseberg, J; Lockman, W S; Nesom, G; Schalk, T; Schmitz, R E; Schumm, B A; Seiden, A; Spradlin, P; Williams, D C; Wilson, M G; Albert, J; Chen, E; Dvoretskii, A; Fang, F; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Ryd, A; Samuel, A; Mancinelli, G; Meadows, B T; Sokoloff, M D; Blanc, F; Bloom, P C; Chen, S; Ford, W T; Hirschauer, J F; Kreisel, A; Nauenberg, U; Olivas, A; Ruddick, W O; Smith, J G; Ulmer, K A; Wagner, S R; Zhang, J; Chen, A; Eckhart, E A; Soffer, A; Toki, W H; Wilson, R J; Winklmeier, F; Zeng, Q; Altenburg, D D; Feltresi, E; Hauke, A; Jasper, H; Petzold, A; Spaan, B; Brandt, T; Klose, V; Lacker, H M; Mader, W F; Nogowski, R; Schubert, J; Schubert, K R; Schwierz, R; Sundermann, J E; Volk, A; Bernard, D; Bonneaud, G R; Grenier, P; Latour, E; Thiebaux, Ch; Verderi, M; Bard, D J; Clark, P J; Gradl, W; Muheim, F; Playfer, S; Robertson, A I; Xie, Y; Andreotti, M; Bettoni, D; Bozzi, C; Calabrese, R; Cibinetto, G; Luppi, E; Negrini, M; Petrella, A; Piemontese, L; Prencipe, E; Anulli, F; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Pacetti, S; Patteri, P; Peruzzi, I M; Piccolo, M; Rama, M; Zallo, A; Buzzo, A; Capra, R; Contri, R; Lo Vetere, M; Macri, M M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Santroni, A; Tosi, S; Brandenburg, G; Chaisanguanthum, K S; Morii, M; Wu, J; Dubitzky, R S; Marks, J; Schenk, S; Uwer, U; Bhimji, W; Bowerman, D A; Dauncey, P D; Egede, U; Flack, R L; Nash, J A; Nikolich, M B; Panduro Vazquez, W; Chai, X; Charles, M J; Mallik, U; Meyer, N T; Ziegler, V; Cochran, J; Crawley, H B; Dong, L; Eyges, V; Meyer, W T; Prell, S; Rosenberg, E I; Rubin, A E; Gritsan, A V; Fritsch, M; Schott, G; Arnaud, N; Davier, M; Grosdidier, G; Höcker, A; Le Diberder, F; Lepeltier, V; Lutz, A M; Oyanguren, A; Pruvot, S; Rodier, S; Roudeau, P; Schune, M H; Stocchi, A; Wang, W F; Wormser, G; Cheng, C H; Lange, D J; Wright, D M; Chavez, C A; Forster, I J; Fry, J R; Gabathuler, E; Gamet, R; George, K A; Hutchcroft, D E; Payne, D J; Schofield, K C; Touramanis, C; Bevan, A J; Di Lodovico, F; Menges, W; Sacco, R; Cowan, G; Flaecher, H U; Hopkins, D A; Jackson, P S; McMahon, T R; Ricciardi, S; Salvatore, F; Wren, A C; Brown, D N; Davis, C L; Allison, J; Barlow, N R; Barlow, R J; Chia, Y M; Edgar, C L; Lafferty, G D; Naisbit, M T; Williams, J C; Yi, J I; Chen, C; Hulsbergen, W D; Jawahery, A; Lae, C K; Roberts, D A; Simi, G; Blaylock, G; Dallapiccola, C; Hertzbach, S S; Li, X; Moore, T B; Saremi, S; Staengle, H; Cowan, R; Sciolla, G; Sekula, S J; Spitznagel, M; Taylor, F; Yamamoto, R K; Kim, H; Patel, P M; Robertson, S H; Lazzaro, A; Lombardo, V; Palombo, F; Bauer, J M; Cremaldi, L; Eschenburg, V; Godang, R; Kroeger, R; Sanders, D A; Summers, D J; Zhao, H W; Brunet, S; Côté, D; Taras, P; Viaud, F B; Nicholson, H; Cavallo, N; De Nardo, G; Fabozzi, F; Gatto, C; Lista, L; Monorchio, D; Paolucci, P; Piccolo, D; Sciacca, C; Baak, M; Raven, G; Snoek, H L; Jessop, C P; LoSecco, J M; Allmendinger, T; Benelli, G; Gan, K K; Honscheid, K; Hufnagel, D; Jackson, P D; Kagan, H; Kass, R; Rahimi, A M; Ter-Antonyan, R; Wong, Q K; Blount, N L; Brau, J; Frey, R; Igonkina, O; Lu, M; Potter, C T; Rahmat, R; Sinev, N B; Strom, D; Strube, J; Torrence, E; Galeazzi, F; Gaz, A; Margoni, M; Morandin, M; Pompili, A; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Voci, C; Benayoun, M; Chauveau, J; David, P; Del Buono, L; de la Vaissière, Ch; Hamon, O; Hartfiel, B L; John, M J J; Malclès, J; Ocariz, J; Roos, L; Therin, G; Behera, P K; Gladney, L; Panetta, J; Biasini, M; Covarelli, R; Angelini, C; Batignani, G; Bettarini, S; Bucci, F; Calderini, G; Carpinelli, M; Cenci, R; Forti, F; Giorgi, M A; Lusiani, A; Marchiori, G; Mazur, M A; Morganti, M; Neri, N; Paoloni, E; Rizzo, G; Walsh, J J; Haire, M; Judd, D; Wagoner, D E; Biesiada, J; Danielson, N; Elmer, P; Lau, Y P; Lu, C; Olsen, J; Smith, A J S; Telnov, A V; Bellini, F; Cavoto, G; D'Orazio, A; del Re, D; Di Marco, E; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Li Gioi, L; Mazzoni, M A; Morganti, S; Piredda, G; Polci, F; Safai Tehrani, F; Voena, C; Ebert, M; Schröder, H; Waldi, R; Adye, T; De Groot, N; Franek, B; Olaiya, E O; Wilson, F F; Aleksan, R; Emery, S; Gaidot, A; Ganzhur, S F; Hamel de Monchenault, G; Kozanecki, W; Legendre, M; Vasseur, G; Yèche, Ch; Zito, M; Chen, X R; Liu, H; Park, W; Purohit, M V; Wilson, J R; Allen, M T; Aston, D; Bartoldus, R; Bechtle, P; Berger, N; Claus, R; Coleman, J P; Convery, M R; Cristinziani, M; Dingfelder, J C; Dorfan, J; Dubois-Felsmann, G P; Dujmic, D; Dunwoodie, W; Field, R C; Glanzman, T; Gowdy, S J; Graham, M T; Halyo, V; Hast, C; Hryn'ova, T; Innes, W R; Kelsey, M H; Kim, P; Leith, D W G S; Li, S; Libby, J; Luitz, S; Luth, V; Lynch, H L; MacFarlane, D B; Marsiske, H; Messner, R; Muller, D R; O'Grady, C P; Ozcan, V E; Perazzo, A; Perl, M; Pulliam, T; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Snyder, A; Stelzer, J; Su, D; Sullivan, M K; Suzuki, K; Swain, S K; Thompson, J M; Tinslay, J S; Va'vra, J; van Bakel, N; Weaver, M; Weinstein, A J R; Wisniewski, W J; Wittgen, M; Wright, D H; Yarritu, A K; Yi, K; Young, C C; Burchat, P R; Edwards, A J; Majewski, S A; Petersen, B A; Roat, C; Wilden, L; Ahmed, S; Alam, M S; Bula, R; Ernst, J A; Jain, V; Pan, B; Saeed, M A; Wappler, F R; Zain, S B; Bugg, W; Krishnamurthy, M; Spanier, S M; Eckmann, R; Ritchie, J L; Satpathy, A; Schilling, C J; Schwitters, R F; Izen, J M; Lou, X C; Ye, S; Bianchi, F; Gallo, F; Gamba, D; Bomben, M; Bosisio, L; Cartaro, C; Cossutti, F; Della Ricca, G; Dittongo, S; Lanceri, L; Vitale, L; Azzolini, V; Martinez-Vidal, F; Banerjee, Sw; Bhuyan, B; Brown, C M; Fortin, D; Hamano, K; Kowalewski, R; Nugent, I M; Roney, J M; Sobie, R J; Back, J J; Harrison, P F; Latham, T E; Mohanty, G B; Pappagallo, M; Band, H R; Chen, X; Cheng, B; Dasu, S; Datta, M; Flood, K T; Hollar, J J; Kutter, P E; Mellado, B; Mihalyi, A; Pan, Y; Pierini, M; Prepost, R; Wu, S L; Yu, Z; Neal, H

    2006-10-27

    The photon spectrum in B-->Xs gamma decay, where Xs is any strange hadronic state, is studied using a data sample of 88.5 x 10(6) e+ e- --> Upsilon(4S) --> BB decays collected by the BABAR experiment at the Stanford Linear Accelerator Center. The partial branching fraction, DeltaB(B --> Xs gamma) = (3.67+/-0.29(stat)+/-0.34(syst)+/-0.29(model)) x 10(-4), the first moment gamma> = 2.288+/-0.025+/-0.017+/-0.015 GeV, and the second moment E2(gamma) = 0.0328+/-0.0040+/-0.0023+/-0.0036 GeV2 are measured for the photon energy range 1.9 GeV < E gamma < 2.7 GeV. They are also measured for narrower E gamma ranges. The moments are then fit to recent theoretical calculations to extract the heavy quark expansion parameters m(b) and mu2(pi) and to extrapolate the partial branching fraction to E gamma > 1.6 GeV. In addition, the direct CP asymmetry A(CP)(B-->X(s+d gamma) is measured to be -0.110+/-0.115(stat)+/-0.017(syst).

  7. Recent Measurements of DT Gamma to Neutron Branching Ratio at ICF Conditions

    NASA Astrophysics Data System (ADS)

    Kim, Yongho

    2011-10-01

    The total T(d,g)5He/T(d,n)4He branching ratio of (4.5 +/- 0.5)E-5 has been measured on Inertial Confinement Fusion (ICF) implosions at the OMEGA laser facility. Recent measurements have shown that the DT branching ratio at ICF is 2 - 3 times less than that of previously measured at particle accelerator facilities. Measurements were done at ion temperatures of (5 +/- 2) keV, which is quite low compared to previous measurements. Implication of the recent founding is that nuclear properties such as DT branching ratio might be reconsidered at low temperature ICF and stellar conditions. In practical sense, precise measurements of the branching ratio T(d,g)5He relative to T(d,n)4He are important in order to diagnose target areal density and resultant fusion yield of cryogenically-layered implosions at the National Ignition Facility (NIF). In this work, we have used LANL's Gas Cherenkov Detector (GCD), which provides a high bandwidth, energy thresholding capability for gamma-ray detection using gamma/electron/Cherenkov conversion. High-bandwidth aids the detection of D-T fusion gamma rays before the arrival of associated 14.1 MeV neutron-induced gammas; energy thresholding gives further protection against such undesirable backgrounds. In addition, to reduce systematic uncertainty, we have applied three independent calibration methods to characterize GCD response such as (1) D-3He gamma-rays generated at Omega laser where no absolute detector calibration was required because quite similar gamma spectrum from D3He and DT, (2) mono-energetic gamma rays generated at Duke University's High Intensity Gamma-ray Source (HIgS), and (3) 14-MeV neutron-induced inelastic gamma-rays generated at OMEGA using puck materials of known areal density placed near target center. In conjunction with an independent neutron yield measurements and ACCEPT and GEANT4 simulation codes, the resultant DT branching ratio was inferred. This work was performed by Los Alamos National Laboratory under the

  8. In situ measurements of thermospheric composition, temperature, and winds by mass spectrometry

    NASA Technical Reports Server (NTRS)

    Spencer, N. W.; Carignan, G. R.

    1988-01-01

    Mass spectrometry, in which a beam of electrons ionizes a sample of atmospheric gas and then analyses the ions thus produced to determine the concentration of each species in the sample, is presently evaluated as a basis for the study of earth atmosphere and other planetary atmospheres' properties. Recent applications of in situ mass spectrometry have measured thermospheric neutral gas composition, temperatures, and winds, with a spatial resolution sufficiently high to reveal previously unsuspected atmospheric variability. It is expected that analyses of these data will lead to a more detailed understanding of the deposition processes governing the thermosphere's highly variable structure.

  9. Decay Heat Measurements Using Total Absorption Gamma-ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Rice, S.; Valencia, E.; Algora, A.; Taín, J. L.; Regan, P. H.; Podolyák, Z.; Agramunt, J.; Gelletly, W.; Nichols, A. L.

    2012-09-01

    A knowledge of the decay heat emitted by thermal neutron-irradiated nuclear fuel is an important factor in ensuring safe reactor design and operation, spent fuel removal from the core, and subsequent storage prior to and after reprocessing, and waste disposal. Decay heat can be readily calculated from the nuclear decay properties of the fission products, actinides and their decay products as generated within the irradiated fuel. Much of the information comes from experiments performed with HPGe detectors, which often underestimate the beta feeding to states at high excitation energies. This inability to detect high-energy gamma emissions effectively results in the derivation of decay schemes that suffer from the pandemonium effect, although such a serious problem can be avoided through application of total absorption γ-ray spectroscopy (TAS). The beta decay of key radionuclei produced as a consequence of the neutron-induced fission of 235U and 239Pu are being re-assessed by means of this spectroscopic technique. A brief synopsis is given of the Valencia-Surrey (BaF2) TAS detector, and their method of operation, calibration and spectral analysis.

  10. Precise atomic mass measurements by deflection mass spectrometry

    NASA Astrophysics Data System (ADS)

    Barber, R. C.; Sharma, K. S.

    2003-05-01

    Since its inception nearly 90 years ago by J.J. Thomson, the precise determination of atomic masses by the classical technique of deflecting charged particles in electric and magnetic fields has provided a large body of data on naturally occurring nuclides. Currently, such measurements on stable nuclides have frequently achieved a precision of better than two parts in 10 9 of the mass. A review of the technique, together with a brief summary of the important historical developments in the field of precise atomic mass measurements, will be given. The more recent contributions to this field by the deflection mass spectrometer at the University of Manitoba will be provided as illustrations of the culmination of the techniques used and the applications that have been studied. A brief comparison between this and newer techniques using Penning traps will be presented.

  11. Servo-amplifiers for ion current measurement in mass spectrometry

    USGS Publications Warehouse

    Stacey, J.S.; Russell, R.D.; Kollar, F.

    1965-01-01

    A servo-voltmeter can provide a useful alternative to the d.c. amplifier or vibrating reed electrometer for the accurate measurement of mass spectrometer ion currents, and has some advantages which recommend its use in certain applications. A generalized analysis based on servomechanism theory is presented as an aid for understanding the design criteria for this type of device. Two existing systems are described and their operation and performance are examined.

  12. Neutral beam species measurements using in situ Rutherford backscatter spectrometry

    SciTech Connect

    Kugel, H.W.; Kaita, R.; Gammel, G.; Williams, M.D.

    1984-12-01

    This work describes a new in situ method for measuring the neutral particle fractions in high power deuterium neutral beams, used to heat magnetically confined fusion plasmas. Deuterium beams, of variable energies, pulse lengths, and powers up to 47 keV, 100 msec, 1.6 MW, were Rutherford backscattered at 135/sup 0/ from TiC inner neutral beam armor of the PDX, and detected using an electrostatic analyzer with microchannel plates. Complete energy scans were made every 20 msec and data were obtained simultaneously from five different positions across the beam profile. The neutral particle fractions were measured to be D/sup 0/(E):D/sup 0/(E/2):D/sup 0/(E/3)=53:32:15. The corresponding neutral power fractions were P/sup 0/(E):P/sup 0/(E/2):P/sup 0/(E/3)=72:21:7, and the associated ionic fractions at the output of the ion source were D/sub 1//sup +/(E):D/sub 2//sup +/(E):D/sub 3//sup +/(E)=74:20:6. The measured neutral particle fractions were relatively constant over more than 70% of the beam power distribution. A decrease in the yield of the full energy component in the outer regions of the beam was observed. Other possible experimental configurations and geometries are discussed.

  13. Neutral beam species measurements using in situ Rutherford backscatter spectrometry

    SciTech Connect

    Kugel, H.W.; Kaita, R.; Gammel, G.; Williams, M.D.

    1985-05-01

    This work describes a new in situ method for measuring the neutral particle fractions in high-power deuterium neutral beams, used to heat magnetically confined fusion plasmas. Deuterium beams, of variable energies, pulse lengths, and powers up to 47 keV, 100 ms, 1.6 MW, were Rutherford backscattered at 135/sup 0/ from the TiC inner neutral beam armor of the PDX, and detected using an electrostatic analyzer with a microchannel plate. Complete energy scans were made every 20 ms and data were obtained simultaneously from five different positions across the beam profile. The neutral particle fractions were measured to be D/sup 0/(E):D/sup 0/(E/2):D/sup 0/(E/3) = 53:32:15. The corresponding neutral power fractions were P/sup 0/(E):P/sup 0/(E/2):P/sup 0/(E/3) = 72:21:7, and the associated ionic fractions at the output of the ion source were D/sup +//sub 1/ (E):D/sup +//sub 2/ (E):D/sup +//sub 3/ (E) = 74:20:6. The measured neutral particle fractions were relatively constant over more than 70% of the beam power distribution. A decrease in the yield of the full-energy component in the outer regions of the beam was observed.

  14. Neutral beam species measurements using in situ Rutherford backscatter spectrometry

    NASA Astrophysics Data System (ADS)

    Kugel, H. W.; Kaita, R.; Gammel, G.; Williams, M. D.

    1985-05-01

    This work describes a new in situ method for measuring the neutral particle fractions in high-power deuterium neutral beams, used to heat magnetically confined fusion plasmas. Deuterium beams, of variable energies, pulse lengths, and powers up to 47 keV, 100 ms, 1.6 MW, were Rutherford backscattered at 135° from the TiC inner neutral beam armor of the PDX, and detected using an electrostatic analyzer with a microchannel plate. Complete energy scans were made every 20 ms and data were obtained simultaneously from five different positions across the beam profile. The neutral particle fractions were measured to be D0(E):D0(E/2):D0(E/3)=53:32:15. The corresponding neutral power fractions were P0(E):P0(E/2):P0(E/3)=72:21:7, and the associated ionic fractions at the output of the ion source were D+1 (E):D+2 (E):D+3 (E)=74:20:6. The measured neutral particle fractions were relatively constant over more than 70% of the beam power distribution. A decrease in the yield of the full-energy component in the outer regions of the beam was observed.

  15. In situ measurements of the sub-surface gamma dose from Chernobyl fallout.

    PubMed

    Timms, D N; Smith, J T; Coe, E; Kudelsky, A V; Yankov, A I

    2005-06-01

    Methods of estimating external radiation exposure of soil-dwelling organisms are currently of much research and regulatory interest. In this paper, we report the first in situ measurements of the sub-surface gamma dose rate for 137Cs contaminated land that quantify variation in dose rate with depth. Two contrasting sites have been investigated. The first site comprised a mineral type soil with a low percentage of organic matter and the second site chosen was in a peat-bog. The different soil compositions afford different 137Cs mobility and this results in variations in the measured gamma dose-rate with soil depth. For each site the paper reports the measured dose rates, the 137Cs activity depth profile, the 137Cs inventory and a description of the soil-characteristics. It is suggested that these data can be used to produce estimates of the sub-surface gamma dose rate in other sites of 137Cs contamination. PMID:15799871

  16. Boron concentration measurement in biological tissues by charged particle spectrometry.

    PubMed

    Bortolussi, S; Altieri, S

    2013-11-01

    Measurement of boron concentration in biological tissues is a fundamental aspect of boron neutron capture therapy, because the outcome of the therapy depends on the distribution of boron at a cellular level, besides on its overall concentration. This work describes a measurement technique based on the spectroscopy of the charged particles emitted in the reaction (10)B(n,α)(7)Li induced by thermal neutrons, allowing for a quantitative determination of the boron concentration in the different components that may be simultaneously present in a tissue sample, such as healthy cells, tumor cells and necrotic cells. Thin sections of tissue containing (10)B are cut at low temperatures and irradiated under vacuum in a thermal neutron field. The charged particles arising from the sample during the irradiation are collected by a thin silicon detector, and their spectrum is used to determine boron concentration through relatively easy calculations. The advantages and disadvantages of this technique are here described, and validation of the method using tissue standards with known boron concentrations is presented.

  17. Modeling of neutron spectrum in the gamma spectroscopy measurements with Ge-detectors

    NASA Astrophysics Data System (ADS)

    Knežević, D.; Jovančević, N.; Krmar, M.; Petrović, J.

    2016-10-01

    In this study, we present a novel approach for estimation of neutron spectra that are present during gamma spectroscopy measurements performed by a Ge detector. This method is based on the calculation of the neutron spectra by using an unfolding procedure, where the activity of the Ge isotopes, produced by the neutron reactions, and the available cross section data for those reactions are the input parameters. This new approach was tested by background gamma spectroscopy measurements with a HPGe detector. Obtained results show that this method can provide useful information about the neutron spectra at the position of the Ge detectors.

  18. Identification and Quantitative Measurements of Chemical Species by Mass Spectrometry

    NASA Technical Reports Server (NTRS)

    Zondlo, Mark A.; Bomse, David S.

    2005-01-01

    The development of a miniature gas chromatograph/mass spectrometer system for the measurement of chemical species of interest to combustion is described. The completed system is a fully-contained, automated instrument consisting of a sampling inlet, a small-scale gas chromatograph, a miniature, quadrupole mass spectrometer, vacuum pumps, and software. A pair of computer-driven valves controls the gas sampling and introduction to the chromatographic column. The column has a stainless steel exterior and a silica interior, and contains an adsorbent of that is used to separate organic species. The detection system is based on a quadrupole mass spectrometer consisting of a micropole array, electrometer, and a computer interface. The vacuum system has two miniature pumps to maintain the low pressure needed for the mass spectrometer. A laptop computer uses custom software to control the entire system and collect the data. In a laboratory demonstration, the system separated calibration mixtures containing 1000 ppm of alkanes and alkenes.

  19. Attogram measurement of rare isotopes by CW resonance ionization mass spectrometry

    SciTech Connect

    Bushaw, B.A.

    1992-05-01

    Three-color double-resonance ionization mass spectrometry, using two single-frequency cw dye lasers and a cw carbon dioxide laser, has been applied to the detection of attogram quantities of rare radionuclides. {sup 210}Pb has been measured in human hair and brain tissue samples to assess indoor radon exposure. Measurements on {sup 90}Sr have shown overall isotopic selectivity of greater than 10{sup 9} despite unfavorable isotope shifts relative to the major stable isotope, {sup 88}Sr.

  20. Photothermal lens spectrometry measurements in highly turbid media.

    PubMed

    Marcano, Aristides; Basaldua, Isaac; Villette, Aaron; Edziah, Raymond; Liu, Jinjie; Ziane, Omar; Melikechi, Noureddine

    2013-09-01

    We measured the photothermal lens signal in samples exhibiting high turbidity using a pump-probe scheme. We show that the photothermal lens signal properties remain nearly unchanged up to values of turbidity of 6 cm(-1) despite the signal reduction due to the decrease of excitation power associated to turbidity losses. The signal starts decreasing abruptly for values of turbidity larger than 6 cm(-1). Multiple light scattering yields a reduction of the temperature gradients, which results in a decrease of the effective signal. However, the signal-to-noise ratio remains above 50 for turbidity values of 9 cm(-1), which corresponds to a reduction of light transmission by more than four orders of magnitude. We report on the detection of the photothermal lens signal through a 2 mm layer of organic tissue with a signal-to-noise ratio of about 500. This technique appears promising for imaging applications in organic samples, which usually exhibit high turbidity for visible and near-infrared light.

  1. Radionuclides in the ground-level atmosphere in Vilnius, Lithuania, in March 2011, detected by gamma-ray spectrometry.

    PubMed

    Gudelis, A; Druteikienė, R; Lujanienė, G; Maceika, E; Plukis, A; Remeikis, V

    2012-07-01

    This study presents the ground-level air monitoring results obtained in Vilnius, the capital of Lithuania, on 14 March-14 April 2011 after the recent earthquake and subsequent Tsunami having a crucial impact on Japanese nuclear reactors at the Fukushima Daiichi Nuclear Power Plant (NPP) on 11 March 2011. To collect representative diurnal aerosol samples a powerful sampling system ensuring the air filtration rate of 5500 m(3) h(-1) was used. The following artificial gamma-ray emitting radionuclides have been determined: (129m)Te, (132)Te (in equilibrium with its daughter (132)I), (131)I, (134)Cs, (136)Cs and (137)Cs. Activity concentration of the globally distributed fission product (137)Cs has increased from a background value of 1.6 μBq m(-3) to the value of 0.9 mBq m(-3) at the beginning of April. The activity ratio (134)Cs/(137)Cs was found to be close to 1, with a slightly higher activity of (134)Cs. The maximum aerosol-associated (131)I activity concentration of 3.45 mBq m(-3) was by four orders of magnitude lower than that measured at the same location in April-May 1986 as a consequence of the Chernobyl NPP accident. The estimated gaseous fraction of iodine-131 constituted about 70% of the total (131)I activity.

  2. Collimated prompt gamma TOF measurements with multi-slit multi-detector configurations

    NASA Astrophysics Data System (ADS)

    Krimmer, J.; Chevallier, M.; Constanzo, J.; Dauvergne, D.; De Rydt, M.; Dedes, G.; Freud, N.; Henriquet, P.; La Tessa, C.; Létang, J. M.; Pleskač, R.; Pinto, M.; Ray, C.; Reithinger, V.; Richard, M. H.; Rinaldi, I.; Roellinghoff, F.; Schuy, C.; Testa, E.; Testa, M.

    2015-01-01

    Longitudinal prompt-gamma ray profiles have been measured with a multi-slit multi-detector configuration at a 75 MeV/u 13C beam and with a PMMA target. Selections in time-of-flight and energy have been applied in order to discriminate prompt-gamma rays produced in the target from background events. The ion ranges which have been extracted from each individual detector module agree amongst each other and are consistent with theoretical expectations. In a separate dedicated experiment with 200 MeV/u 12C ions the fraction of inter-detector scattering has been determined to be on the 10%-level via a combination of experimental results and simulations. At the same experiment different collimator configurations have been tested and the shielding properties of tungsten and lead for prompt-gamma rays have been measured.

  3. Evaluation of the measurement geometries and data processing algorithms for industrial gamma tomography technology.

    PubMed

    Lee, N Y; Jung, S H; Kim, J B

    2009-01-01

    In this paper, we evaluated the measurement geometries and data processing algorithms for industrial gamma tomography technology. Several phantoms simulating industrial objects were tested in various conditions with the gamma-ray CT system developed in KAERI (Korea Atomic Energy Research Institute). Radiation was measured with lead shielded 24 1x1in Nal detectors. Regarding the parallel beam geometry, the EM algorithm showed the best resolution among the algebraic reconstruction technique (ART), simultaneous iterative reconstructive technique (SIRT) and expectation maximization (EM). However, the fan beam scanning was more time efficient than the parallel projection for the similar quality of reconstructed image. Future developments of the industrial gamma ray CT will be focused on a large-scale application which is more practical for a diagnosis in the petrochemical industry. PMID:19376727

  4. The Probing In-Situ With Neutron and Gamma Rays (PING) Instrument for Planetary Composition Measurements

    NASA Technical Reports Server (NTRS)

    Parsons, A.; Bodnarik, J.; Evans, L.; McClanahan, T.; Namkung, M.; Nowicki, S.; Schweitzer, J.; Starr, R.

    2012-01-01

    The Probing In situ with Neutrons and Gamma rays (PING) instrument (formerly named PNG-GRAND) [I] experiment is an innovative application of the active neutron-gamma ray technology successfully used in oil field well logging and mineral exploration on Earth over many decades. The objective of our active neutron-gamma ray technology program at NASA Goddard Space Flight Center (NASA/GSFC) is to bring PING to the point where it can be flown on a variety of surface lander or rover missions to the Moon, Mars, Venus, asteroids, comets and the satellites of the outer planets and measure their bulk surface and subsurface elemental composition without the need to drill into the surface. Gamma-Ray Spectrometers (GRS) have been incorporated into numerous orbital planetary science missions. While orbital measurements can map a planet, they have low spatial and elemental sensitivity due to the low surface gamma ray emission rates reSUlting from using cosmic rays as an excitation source, PING overcomes this limitation in situ by incorporating a powerful neutron excitation source that permits significantly higher elemental sensitivity elemental composition measurements. PING combines a 14 MeV deuterium-tritium Pulsed Neutron Generator (PNG) with a gamma ray spectrometer and two neutron detectors to produce a landed instrument that can determine the elemental composition of a planet down to 30 - 50 cm below the planet's surface, The penetrating nature of .5 - 10 MeV gamma rays and 14 MeV neutrons allows such sub-surface composition measurements to be made without the need to drill into or otherwise disturb the planetary surface, thus greatly simplifying the lander design, We are cun'ently testing a PING prototype at a unique outdoor neutron instrumentation test facility at NASA/GSFC that provides two large (1.8 m x 1.8 m x ,9 m) granite and basalt test formations placed outdoors in an empty field, Since an independent trace elemental analysis has been performed on both these

  5. The use of MCNP and gamma spectrometry in supporting the evaluation of NORM in Libyan oil pipeline scale

    NASA Astrophysics Data System (ADS)

    Habib, Ahmed S.; Bradley, D. A.; Regan, P. H.; Shutt, A. L.

    2010-07-01

    The accumulation of scales in production pipes is a common problem in the oil industry, reducing fluid flow and also leading to costly remedies and disposal issues. Typical materials found in such scale are sulphates and carbonates of calcium and barium, or iron sulphide. Radium arising from the uranium/thorium present in oil-bearing rock formations may replace the barium or calcium in these salts to form radium salts. This creates what is known as technologically enhanced naturally occurring radioactive material (TENORM or simply NORM). NORM is a serious environmental and health and safety issue arising from commercial oil and gas extraction operations. Whilst a good deal has been published on the characterisation and measurement of radioactive scales from offshore oil production, little information has been published regarding NORM associated with land-based facilities such as that of the Libyan oil industry. The ongoing investigation described in this paper concerns an assessment of NORM from a number of land based Libyan oil fields. A total of 27 pipe scale samples were collected from eight oil fields, from different locations in Libya. The dose rates, measured using a handheld survey meter positioned on sample surfaces, ranged from 0.1-27.3 μSv h -1. In the initial evaluations of the sample activity, use is being made of a portable HPGe based spectrometry system. To comply with the prevailing safety regulations of the University of Surrey, the samples are being counted in their original form, creating a need for correction of non-homogeneous sample geometries. To derive a detection efficiency based on the actual sample geometries, a technique has been developed using a Monte Carlo particle transport code (MCNPX). A preliminary activity determination has been performed using an HPGe portable detector system.

  6. Measurement of the {sup 241}Am({gamma},n){sup 240}Am reaction in the giant dipole resonance region

    SciTech Connect

    Tonchev, A. P.; Howell, C. R.; Hutcheson, A.; Kwan, E.; Raut, R.; Rusev, G.; Tornow, W.; Hammond, S. L.; Huibregtse, C.; Kelley, J. H.; Kawano, T.; Vieira, D. J.; Wilhelmy, J. B.

    2010-11-15

    The photodisintegration cross section of the radioactive nucleus {sup 241}Am has been obtained using activation techniques and monoenergetic {gamma}-ray beams from the HI{gamma}S facility. The induced activity of {sup 240}Am produced via the {sup 241}Am({gamma},n) reaction was measured in the energy interval from 9 to 16 MeV utilizing high-resolution {gamma}-ray spectroscopy. The experimental data for the {sup 241}Am({gamma},n) reaction in the giant dipole resonance energy region are compared with statistical nuclear-model calculations.

  7. Measurement of Relative Dissolved Gas Concentrations Using Underwater Mass Spectrometry

    NASA Astrophysics Data System (ADS)

    Bell, R. J.; Toler, S.; van Amerom, F. H.; Wenner, P.; Hall, M.; Edkins, J.; Gassig, S.; Short, R.; Byrne, R.

    2004-12-01

    -gas compositions at different sites point to diverse geothermal conditions beneath the lake. Oxygen concentrations were low at most vents, while hydrogen sulfide, methane and carbon dioxide concentrations were highly variable. Dissolved gas depth profiles were obtained using the UMS system in Saanich Inlet, Canada. Due to degradation of organic material, the inlet's deep water is typically anoxic, and rich in methane, carbon dioxide, and reduced sulfur compounds. Relative gas concentrations were obtained between the surface and 200m. A thermocline was detected as the instrument entered anoxic bottom water at 100m. Below this depth oxygen signal intensity declined sharply to background levels. In contrast, carbon dioxide increased sharply below 100m until a reproducible maximum was observed at 120m. Methane and hydrogen sulfide increased steadily with depth below 100 m, and exhibited no local maxima. Fully quantitative UMS measurements require characterization of the influence of salinity, and especially temperature and pressure, on the performance of the internal PDMS membrane. Temperature exerts a strong influence on gas diffusion across the PDMS membrane and the behavior of residual gases in the vacuum chamber; therefore, precise thermostating methods must be adopted. Other technical issues being examined in the laboratory include variations in UMS response attributable to pressure-induced membrane compression, and variable hydrodynamic conditions at the sample/membrane boundary. Experiments are being developed to address the issue of calibrating the ion signal intensity for dissolved gas concentrations.

  8. Confidence Intervals for Gamma-Family Measures of Ordinal Association

    ERIC Educational Resources Information Center

    Woods, Carol M.

    2007-01-01

    This research focused on confidence intervals (CIs) for 10 measures of monotonic association between ordinal variables. Standard errors (SEs) were also reviewed because more than 1 formula was available per index. For 5 indices, an element of the formula used to compute an SE is given that is apparently new. CIs computed with different SEs were…

  9. Radiation measurement above the lunar surface by Kaguya gamma-ray spectrometer

    NASA Astrophysics Data System (ADS)

    Hasebe, Nobuyuki; Nagaoka, Hiroshi; Kusano, Hiroki; Hareyama, Matoko; Ideguchi, Yusuke; Shimizu, Sota; Shibamura, Eido

    The lunar surface is filled with various ionizing radiations such as high energy galactic particles, albedo particles and secondary radiations of neutrons, gamma rays and other elementary particles. A high-resolution Kaguya Gamma-Ray Spectrometer (KGRS) was carried on the Japan’s lunar explorer SELENE (Kaguya), the largest lunar orbiter since the Apollo missions. The KGRS instrument employed, for the first time in lunar exploration, a high-purity Ge crystal to increase the identification capability of elemental gamma-ray lines. The Ge detector is surrounded by BGO and plastic counters as for anticoincidence shields. The KGRS measured gamma rays in the energy range from 200 keV to 13 MeV with high precision to determine the chemical composition of the lunar surface. It provided data on the abundance of major elements over the entire lunar surface. In addition to the gamma-ray observation by the KGRS, it successfully measured the global distribution of fast neutrons. In the energy spectra of gamma-rays observed by the KGRS, several saw-tooth- peaks of Ge are included, which are formed by the collision interaction of lunar fast neutrons with Ge atoms in the Ge crystal. With these saw-tooth-peaks analysis, global distribution of neutrons emitted from the lunara surface was successfully created, which was compared with the previous results obtained by Lunar Prospector neutron maps. Another anticoincidence counter, the plastic counter with 5 mm thickness, was used to veto radiation events mostly generated by charged particles. A single photomultiplier serves to count scintillation light from the plastic scintillation counter. The global map of counting rates observed by the plastic counter was also created, implying that the radiation counting rate implies the geological distribution, in spite that the plastic counter mostly measures high energy charged particles and energetic neutrons. These results are presented and discussed.

  10. Measurement of areal density in the ablators of inertial-confinement-fusion capsules via detection of ablator (n, n Prime {gamma}) gamma-ray emission

    SciTech Connect

    Hoffman, N. M.; Herrmann, H. W.; Kim, Y. H.; Hsu, H. H.; Young, C. S.; Mack, J. M.; Wilson, D. C.; Langenbrunner, J. R.; Evans, S. C.; Sedillo, T. J.; Horsfield, C. J.; Rubery, M. S.; Miller, E. K.; Grafil, E.; Stoeffl, W.; Church, J. A.; Glebov, V. Yu.; Duffy, T.

    2013-04-15

    We report the first gamma-ray-based measurements of the areal density of ablators in inertial-confinement-fusion capsule implosions. The measurements, made at the OMEGA laser [T. R. Boehly et al., Opt. Commun. 133, 495 (1997)], used observations of gamma rays arising from inelastic scattering of 14.1-MeV deuterium-tritium (DT) neutrons on {sup 12}C nuclei in the compressed plastic ablators. The emission of {sup 12}C(n,n Prime {gamma}) gamma rays from the capsules is detected using the Gamma Reaction History instrument [H. W. Herrmann et al., J. Phys.: Conf. Ser. 244, 032047 (2010)] operating at OMEGA. From the ratio of a capsule's {sup 12}C(n,n Prime {gamma}) emission to the emission from the same processes in an in situ reference graphite 'puck' of known mass and geometry [N. M. Hoffman et al., in IFSA 2011 proceedings (submitted)], we determine the time-averaged areal density of {sup 12}C in the capsule's compressed ablator. Measured values of total ablator areal density for thirteen imploded capsules, in the range 23 {+-} 10 to 58 {+-} 14 mg/cm{sup 2}, are comparable to values calculated in 1D radiation-hydrodynamic simulations, and measured by charged-particle techniques.

  11. Gamma-Ray Attenuation Measurements as a Laboratory Experiment: Some Remarks

    ERIC Educational Resources Information Center

    Adamides, E.; Koutroubas, S. K.; Moshonas, N.; Yiasemides, K.

    2011-01-01

    In this article we make some significant remarks on the experimental study of the absorption of gamma radiation passing through matter. These remarks have to do with the seemingly unexpected trend of the measured intensity of radiation versus the thickness of the absorber, which puzzles students and its explanation eludes many laboratory…

  12. Measurement of gamma and neutron radiations inside spent fuel assemblies with passive detectors

    NASA Astrophysics Data System (ADS)

    Viererbl, L.; Lahodová, Z.; Voljanskij, A.; Klupák, V.; Koleška, M.; Cabalka, M.; Turek, K.

    2011-10-01

    During operation of a fission nuclear reactor, many radionuclides are generated in fuel by fission and activation of 235U, 238U and other nuclides present in the assembly. After removal of a fuel assembly from the core, these radionuclides are sources of different types of radiation. Gamma and neutron radiation emitted from an assembly can be non-destructively detected with different types of detectors. In this paper, a new method of measurement of radiation from a spent fuel assembly is presented. It is based on usage of passive detectors, such as alanine dosimeters for gamma radiation and track detectors for neutron radiation. Measurements are made on the IRT-2M spent fuel assemblies used in the LVR-15 research reactor. During irradiation of detectors, the fuel assembly is located in a water storage pool at a depth of 6 m. Detectors are inserted into central hole of the assembly, irradiated for a defined time interval, and after the detectors removed from the assembly, gamma dose or neutron fluence are evaluated. Measured profiles of gamma dose rate and neutron fluence rate inside of the spent fuel assembly are presented. This measurement can be used to evaluate relative fuel burn-up.

  13. "Confidence Intervals for Gamma-family Measures of Ordinal Association": Correction

    ERIC Educational Resources Information Center

    Psychological Methods, 2008

    2008-01-01

    Reports an error in "Confidence intervals for gamma-family measures of ordinal association" by Carol M. Woods (Psychological Methods, 2007[Jun], Vol 12[2], 185-204). The note corrects simulation results presented in the article concerning the performance of confidence intervals (CIs) for Spearman's r-sub(s). An error in the author's C++ code…

  14. MEG sensor and source measures of visually induced gamma-band oscillations are highly reliable.

    PubMed

    Tan, H-R M; Gross, J; Uhlhaas, P J

    2016-08-15

    High frequency brain oscillations are associated with numerous cognitive and behavioral processes. Non-invasive measurements using electro-/magnetoencephalography (EEG/MEG) have revealed that high frequency neural signals are heritable and manifest changes with age as well as in neuropsychiatric illnesses. Despite the extensive use of EEG/MEG-measured neural oscillations in basic and clinical research, studies demonstrating test-retest reliability of power and frequency measures of neural signals remain scarce. Here, we evaluated the test-retest reliability of visually induced gamma (30-100Hz) oscillations derived from sensor and source signals acquired over two MEG sessions. The study required participants (N=13) to detect the randomly occurring stimulus acceleration while viewing a moving concentric grating. Sensor and source MEG measures of gamma-band activity yielded comparably strong reliability (average intraclass correlation, ICC=0.861). Peak stimulus-induced gamma frequency (53-72Hz) yielded the highest measures of stability (ICCsensor=0.940; ICCsource=0.966) followed by spectral signal change (ICCsensor=0.890; ICCsource=0.893) and peak frequency bandwidth (ICCsensor=0.856; ICCsource=0.622). Furthermore, source-reconstruction significantly improved signal-to-noise for spectral amplitude of gamma activity compared to sensor estimates. Our assessments highlight that both sensor and source derived estimates of visually induced gamma-band oscillations from MEG signals are characterized by high test-retest reliability, with source derived oscillatory measures conferring an improvement in the stability of peak-frequency estimates. Importantly, our finding of high test-retest reliability supports the feasibility of pharma-MEG studies and longitudinal aging or clinical studies. PMID:27153980

  15. MEG sensor and source measures of visually induced gamma-band oscillations are highly reliable.

    PubMed

    Tan, H-R M; Gross, J; Uhlhaas, P J

    2016-08-15

    High frequency brain oscillations are associated with numerous cognitive and behavioral processes. Non-invasive measurements using electro-/magnetoencephalography (EEG/MEG) have revealed that high frequency neural signals are heritable and manifest changes with age as well as in neuropsychiatric illnesses. Despite the extensive use of EEG/MEG-measured neural oscillations in basic and clinical research, studies demonstrating test-retest reliability of power and frequency measures of neural signals remain scarce. Here, we evaluated the test-retest reliability of visually induced gamma (30-100Hz) oscillations derived from sensor and source signals acquired over two MEG sessions. The study required participants (N=13) to detect the randomly occurring stimulus acceleration while viewing a moving concentric grating. Sensor and source MEG measures of gamma-band activity yielded comparably strong reliability (average intraclass correlation, ICC=0.861). Peak stimulus-induced gamma frequency (53-72Hz) yielded the highest measures of stability (ICCsensor=0.940; ICCsource=0.966) followed by spectral signal change (ICCsensor=0.890; ICCsource=0.893) and peak frequency bandwidth (ICCsensor=0.856; ICCsource=0.622). Furthermore, source-reconstruction significantly improved signal-to-noise for spectral amplitude of gamma activity compared to sensor estimates. Our assessments highlight that both sensor and source derived estimates of visually induced gamma-band oscillations from MEG signals are characterized by high test-retest reliability, with source derived oscillatory measures conferring an improvement in the stability of peak-frequency estimates. Importantly, our finding of high test-retest reliability supports the feasibility of pharma-MEG studies and longitudinal aging or clinical studies.

  16. Staying Alive: Measuring Intact Viable Microbes with Electrospray Ionization Mass Spectrometry

    NASA Astrophysics Data System (ADS)

    Forsberg, Erica; Fang, Mingliang; Siuzdak, Gary

    2016-07-01

    Mass spectrometry has traditionally been the technology of choice for small molecule analysis, making significant inroads into metabolism, clinical diagnostics, and pharmacodynamics since the 1960s. In the mid-1980s, with the discovery of electrospray ionization (ESI) for biomolecule analysis, a new door opened for applications beyond small molecules. Initially, proteins were widely examined, followed by oligonucleotides and other nonvolatile molecules. Then in 1991, three intriguing studies reported using mass spectrometry to examine noncovalent protein complexes, results that have been expanded on for the last 25 years. Those experiments also raised the questions: How soft is ESI, and can it be used to examine even more complex interactions? Our lab addressed these questions with the analyses of viruses, which were initially tested for viability following electrospray ionization and their passage through a quadrupole mass analyzer by placing them on an active medium that would allow them to propagate. This observation has been replicated on multiple different systems, including experiments on an even bigger microbe, a spore. The question of analysis was also addressed in the early 2000s with charge detection mass spectrometry. This unique technology could simultaneously measure mass-to-charge and charge, allowing for the direct determination of the mass of a virus. More recent experiments on spores and enveloped viruses have given us insight into the range of mass spectrometry's capabilities (reaching 100 trillion Da), beginning to answer fundamental questions regarding the complexity of these organisms beyond proteins and genes, and how small molecules are integral to these supramolecular living structures.

  17. Statistical Measurement of the Gamma-Ray Source-count Distribution as a Function of Energy

    NASA Astrophysics Data System (ADS)

    Zechlin, Hannes-S.; Cuoco, Alessandro; Donato, Fiorenza; Fornengo, Nicolao; Regis, Marco

    2016-08-01

    Statistical properties of photon count maps have recently been proven as a new tool to study the composition of the gamma-ray sky with high precision. We employ the 1-point probability distribution function of six years of Fermi-LAT data to measure the source-count distribution dN/dS and the diffuse components of the high-latitude gamma-ray sky as a function of energy. To that aim, we analyze the gamma-ray emission in five adjacent energy bands between 1 and 171 GeV. It is demonstrated that the source-count distribution as a function of flux is compatible with a broken power law up to energies of ˜50 GeV. The index below the break is between 1.95 and 2.0. For higher energies, a simple power-law fits the data, with an index of {2.2}-0.3+0.7 in the energy band between 50 and 171 GeV. Upper limits on further possible breaks as well as the angular power of unresolved sources are derived. We find that point-source populations probed by this method can explain {83}-13+7% ({81}-19+52%) of the extragalactic gamma-ray background between 1.04 and 1.99 GeV (50 and 171 GeV). The method has excellent capabilities for constraining the gamma-ray luminosity function and the spectra of unresolved blazars.

  18. 232Th(n,{gamma})233Th Thermal Reaction Cross-Section Measurement

    SciTech Connect

    Maidana, Nora L.; Vanin, Vito R.; Pascholati, Paulo R.; Helene, Otaviano; Castro, Ruy M.; Dias, Mauro S.; Koskinas, Marina F.

    2005-05-24

    The 232Th(n,{gamma})233Th thermal neutron-capture reaction cross section was measured using targets of {approx} 1.5 mg of high-purity metallic thorium irradiated in the IPEN IEA-R1m 5 MW pool research reactor. The 197Au(n,{gamma})198Au reaction was used to monitor the thermal and epithermal neutron fluxes in the irradiation position, which was found using the Westcott formalism. The residual gamma-ray activity was followed with an HPGe detector. The detector efficiency curve was fitted by the least-squares method applying covariance analysis to all uncertainties involved. The experimental result is {sigma}0 =7.20{+-}0.20 b, in agreement with previous published values.

  19. Method and apparatus for measuring incombustible content of coal mine dust using gamma-ray backscatter

    DOEpatents

    Armstrong, Frederick E.

    1976-09-28

    Method and apparatus for measuring incombustible content of particulate material, particularly coal mine dust, includes placing a sample of the particulate material in a container to define a pair of angularly oriented surfaces of the sample, directing an incident gamma-ray beam from a radiation source at one surface of the sample and detecting gamma-ray backscatter from the other surface of the sample with a radiation detector having an output operating a display to indicate incombustible content of the sample. The positioning of the source and detector along different surfaces of the sample permits the depth of the scattering volume defined by intersection of the incident beam and a detection cone from the detector to be selected such that variations in scattered radiation produced by variations in density of the sample are compensated by variations in the attenuation of the incident beam and the gamma-ray backscatter.

  20. Measurement of U-235 Fission Neutron Spectra Using a Multiple Gamma Coincidence Technique

    SciTech Connect

    Ji Chuncheng; Kegel, G.H.R.; Egan, J.J.; DeSimone, D.J.; Alimeti, A.; Roldan, C.F.; McKittrick, T.M.; Kim, D.-S.; Chen, X.; Tremblay, S.E.

    2005-05-24

    The Los Alamos Model of Madland and Nix predicts the shape of the fission neutron energy spectrum for incident primary neutrons of different energies. Verifications of the model normally are limited to measurements of the fission neutron spectra for energies higher than that of the primary neutrons because the low-energy spectrum is distorted by the admixture of elastically and inelastically scattered neutrons. This situation can be remedied by using a measuring technique that separates fission from scattering events. One solution consists of using a fissile sample so thin that fission fragments can be observed indicating the occurrence of a fission event. A different approach is considered in this paper. It has been established that a fission event is accompanied by the emission of between seven and eight gamma rays, while in a scattering interaction, between zero and two gammas are emitted, so that a gamma multiplicity detector should supply a datum to distinguish a fission event from a scattering event. We proceed as follows: A subnanosecond pulsed and bunched proton beam from the UML Van de Graaff generates nearly mono-energetic neutrons by irradiating a thin metallic lithium target. The neutrons irradiate a 235U sample. Emerging neutron energies are measured with a time-of-flight spectrometer. A set of four BaF2 detectors is located close to the 235U sample. These detectors together with their electronic components identify five different events for each neutron detected, i.e., whether four, three, two, one, or none of the BaF2 detectors received one (or more) gamma rays. We present work, preliminary to the final measurements, involving feasibility considerations based on gamma-ray coincidence measurements with four BaF2 detectors, and the design of a Fission-Scattering Discriminator under construction.

  1. Measurement of the Z gamma ---> nu anti-nu gamma cross section and limits on anomalous Z Z gamma and Z gamma gamma couplings in p anti-p collisions at s**(1/2) = 1.96-TeV

    SciTech Connect

    Abazov, V.M.; Abbott, B.; Abolins, M.; Acharya, Bannanje Sripath; Adams, M.; Adams, T.; Aguilo, E.; Ahsan, M.; Alexeev, G.D.; Alkhazov, Georgiy D.; Alton, Andrew K.; /Michigan U. /Northeastern U.

    2009-02-01

    We present the first observation of the Z{gamma} {yields}{nu}{bar {nu}}{gamma} process at the Tevatron at 5.1 standard deviations significance, based on 3.6 fb{sup -1} of integrated luminosity collected with the D0 detector at the Fermilab Tevatron p{bar p} Collider at {radical}s = 1.96 TeV. The measured Z{gamma} cross section multiplied by the branching fraction of Z {yields} {nu}{bar {nu}} is 32 {+-} 9(stat. + syst.) {+-} 2(lumi.) fb for the photon E{sub T} > 90 GeV. It is in agreement with the standard model prediction of 39 {+-} 4 fb. We set the most restrictive limits on anomalous trilinear Z{gamma}{gamma} and ZZ{gamma} gauge boson couplings at a hadron collider to date, with three constraints being the world's strongest.

  2. Testing a Light-weight Compact Gamma Ray Detector for Measuring Snow Water Equivalent

    NASA Astrophysics Data System (ADS)

    Saiet, E., II; Solie, D. J.; Sturm, M.

    2014-12-01

    The use of gamma ray to measure snow water equivalent (SWE) trace back to the 1970s during the Soviet Union hydrology program. Over the years research has shown that gamma detectors could be used to monitor SWE, and their use significantly expanded. In the 1980s several airborne campaigns were launched in North America to measure SWR; these gamma flights are still in use today. However, these airborne flights require a twin-engine aircraft and a detector with a computer that weighs 250 kg, which is unsuitable for use with unmanned airborne systems (UAS), our primary interest. Here we describe results of tests of a compact gamma detector weighing 2 kg. The envisioned deployment of this detector is on a small quad-copter UAS that can hover low over remote clearings in the boreal forest of interior Alaska. Such a technique may allow SWE estimates in places that otherwise would be difficult to measure. We tested the detector over snow and water bodies and found for SWE between 0 and 50 cm a sensitivity of ± 2 cm SWE, which is sufficient to resolve any significant snowfall in the region. In this presentation we will discuss our preliminary results and our future strategy for deploying the sensor on a UAS.

  3. Anisotropies in the Diffuse Gamma-Ray Background Measured by the Fermi LAT

    NASA Technical Reports Server (NTRS)

    Ferrara, E. C.; McEnery, J. E.; Troja, E.

    2012-01-01

    The contribution of unresolved sources to the diffuse gamma-ray background could induce anisotropies in this emission on small angular scales. We analyze the angular power spectrum of the diffuse emission measured by the Fermi LAT at Galactic latitudes absolute value of b > 30 deg in four energy bins spanning 1 to 50 GeV. At multipoles l >= 155, corresponding to angular scales approx < 2 deg, angular power above the photon noise level is detected at > 99.99% CL in the 1-2 GeV, 2- 5 GeV, and 5- 10 GeV energy bins, and at > 99% CL at 10-50 GeV. Within each energy bin the measured angular power takes approximately the same value at all multipoles l >= 155, suggesting that it originates from the contribution of one or more unclustered source populations. The amplitude of the angular power normalized to the mean intensity in each energy bin is consistent with a constant value at all energies, C(sub p) / (I)(exp 2) = 9.05 +/- 0.84 x 10(exp -6) sr, while the energy dependence of C(sub p) is consistent with the anisotropy arising from one or more source populations with power-law photon spectra with spectral index Gamma (sub s) = 2.40 +/- 0.07. We discuss the implications of the measured angular power for gamma-ray source populations that may provide a contribution to the diffuse gamma-ray background.

  4. Radiative Penguin Decays of B Mesons: Measurements of B to K* gamma, B to K2* gamma, and Search for B0 to phi gamma

    SciTech Connect

    Bauer, J.

    2005-01-03

    Electromagnetic radiative penguin decays of the B meson were studied with the BaBar detector at SLAC's PEP-II asymmetric-energy B Factory. Branching fractions and isospin asymmetry of the decay B {yields} K*{gamma}, branching fractions of B {yields} K*{sub 2}(1430){gamma}, and a search for B{sup 0} {yields} {phi}{gamma} are presented. The decay rates may be enhanced by contributions from non-standard model processes.

  5. Neutron and gamma-ray dose measurements at various distances from the Little Boy replica

    SciTech Connect

    Huntzinger, C.J.; Hankins, D.E.

    1984-08-01

    We measured neutron and gamma-ray dose rates at various distances from the Little Boy-Comet Critical Assembly at Los Alamos National Laboratory (LANL) in April of 1983. The Little Boy-Comet Assembly is a replica of the atomic weapon detonated over Hiroshima, designed to be operated at various steady-state power levels. The selected distances for measurement ranged from 107 m to 567 m. Gamma-ray measurements were made with a Reuter-Stokes environmental ionization chamber which has a sensitivity of 1.0 ..mu..R/hour. Neutron measurements were made with a pulsed-source remmeter which has a sensitivity of 0.1 ..mu..rem/hour, designed and built at Lawrence Livermore National Laboratory (LLNL). 12 references, 7 figures, 6 tables.

  6. Gamma Astrometric Measurement Experiment (GAME) - Implementation and performance

    NASA Astrophysics Data System (ADS)

    Gai, Mario; Gai, Mario; Vecchiato, Alberto; Lattanzi, Mario G.; Ligori, Sebastiano; Loreggia, Davide

    The GAME mission concept is aimed at test of the General Relativity, through very precise measurement of the gravitational deflection of light by the Sun, by means of an optimised telescope operating in the visible and launched in orbit on a small class satellite. We recall the science motivations, discussed in detail in a separate contribution by Vecchiato et al., and describe the mission requirements derivation, the proposed mission profile, the preliminary payload design and the expected performance. The targeted precision on the "γ" parameter of the Parametrised Post-Newtonian formulation of General Relativity is in the range 10-6 to 10-7 or better, with an improvement of one or two orders of magnitude with respect to the best currently available experimental results. Such precision is suitable to detect possible deviations of γ from the unity value, associated to generalised Einstein models for gravitation, with potentially huge impacts on the cosmological distribution of dark matter and dark energy. The measurement principle is based on the differential astrometric signature on the stellar positions, i.e. on the spatial component of the gravitational effect, rather than the temporal component as in the most recent experiments based on radio link delay timing. Calibration is based on frequent measurement of angular separation of bright sources in stellar fields affected by negligible deflection. The instrument concept is based on a dual field, multiple aperture Fizeau interferometer, observing simultaneously two sky regions close to the Solar limb. A split flat mirror is used to fold the telescope line of sight on two different directions on the sky, separated by a base angle of about 4 degrees, which represents the gauge applied on the sky to measure the desired angular value of deflection. Stability or calibration of the base angle is the key to fulfilling the GAME science goals. An internal laser metrology option is considered for both on ground

  7. Levels of naturally occurring gamma radiation measured in British homes and their prediction in particular residences.

    PubMed

    Kendall, G M; Wakeford, R; Athanson, M; Vincent, T J; Carter, E J; McColl, N P; Little, M P

    2016-03-01

    Gamma radiation from natural sources (including directly ionising cosmic rays) is an important component of background radiation. In the present paper, indoor measurements of naturally occurring gamma rays that were undertaken as part of the UK Childhood Cancer Study are summarised, and it is shown that these are broadly compatible with an earlier UK National Survey. The distribution of indoor gamma-ray dose rates in Great Britain is approximately normal with mean 96 nGy/h and standard deviation 23 nGy/h. Directly ionising cosmic rays contribute about one-third of the total. The expanded dataset allows a more detailed description than previously of indoor gamma-ray exposures and in particular their geographical variation. Various strategies for predicting indoor natural background gamma-ray dose rates were explored. In the first of these, a geostatistical model was fitted, which assumes an underlying geologically determined spatial variation, superimposed on which is a Gaussian stochastic process with Matérn correlation structure that models the observed tendency of dose rates in neighbouring houses to correlate. In the second approach, a number of dose-rate interpolation measures were first derived, based on averages over geologically or administratively defined areas or using distance-weighted averages of measurements at nearest-neighbour points. Linear regression was then used to derive an optimal linear combination of these interpolation measures. The predictive performances of the two models were compared via cross-validation, using a randomly selected 70 % of the data to fit the models and the remaining 30 % to test them. The mean square error (MSE) of the linear-regression model was lower than that of the Gaussian-Matérn model (MSE 378 and 411, respectively). The predictive performance of the two candidate models was also evaluated via simulation; the OLS model performs significantly better than the Gaussian-Matérn model.

  8. MEASUREMENT OF THE EXPANSION RATE OF THE UNIVERSE FROM {gamma}-RAY ATTENUATION

    SciTech Connect

    Dominguez, Alberto; Prada, Francisco

    2013-07-10

    A measurement of the expansion rate of the universe (that is, the Hubble constant, H{sub 0}) is derived here using the {gamma}-ray attenuation observed in the spectra of {gamma}-ray sources produced by the interaction of extragalactic {gamma}-ray photons with the photons of the extragalactic background light (EBL). The Hubble constant determined with our technique, for a {Lambda}CDM cosmology, is H{sub 0}=71.8{sub -5.6}{sup +4.6}(stat){sub -13.8}{sup +7.2}(syst) km s{sup -1} Mpc{sup -1}. This value is compatible with present-day measurements using well-established methods such as local distance ladders and cosmological probes. The recent detection of the cosmic {gamma}-ray horizon (CGRH) from multiwavelength observations of blazars, together with the advances in the knowledge of the EBL, allow us to measure the expansion rate of the universe. This estimate of the Hubble constant shows that {gamma}-ray astronomy has reached a mature enough state to provide cosmological measurements, which may become more competitive in the future with the construction of the Cherenkov Telescope Array. We find that the maximum dependence of the CGRH on the Hubble constant is approximately between redshifts 0.04 and 0.1, thus this is a smoking gun for planning future observational efforts. Other cosmological parameters, such as the total dark matter density {Omega}{sub m} and the dark energy equation of state w, are explored as well.

  9. Levels of naturally occurring gamma radiation measured in British homes and their prediction in particular residences.

    PubMed

    Kendall, G M; Wakeford, R; Athanson, M; Vincent, T J; Carter, E J; McColl, N P; Little, M P

    2016-03-01

    Gamma radiation from natural sources (including directly ionising cosmic rays) is an important component of background radiation. In the present paper, indoor measurements of naturally occurring gamma rays that were undertaken as part of the UK Childhood Cancer Study are summarised, and it is shown that these are broadly compatible with an earlier UK National Survey. The distribution of indoor gamma-ray dose rates in Great Britain is approximately normal with mean 96 nGy/h and standard deviation 23 nGy/h. Directly ionising cosmic rays contribute about one-third of the total. The expanded dataset allows a more detailed description than previously of indoor gamma-ray exposures and in particular their geographical variation. Various strategies for predicting indoor natural background gamma-ray dose rates were explored. In the first of these, a geostatistical model was fitted, which assumes an underlying geologically determined spatial variation, superimposed on which is a Gaussian stochastic process with Matérn correlation structure that models the observed tendency of dose rates in neighbouring houses to correlate. In the second approach, a number of dose-rate interpolation measures were first derived, based on averages over geologically or administratively defined areas or using distance-weighted averages of measurements at nearest-neighbour points. Linear regression was then used to derive an optimal linear combination of these interpolation measures. The predictive performances of the two models were compared via cross-validation, using a randomly selected 70 % of the data to fit the models and the remaining 30 % to test them. The mean square error (MSE) of the linear-regression model was lower than that of the Gaussian-Matérn model (MSE 378 and 411, respectively). The predictive performance of the two candidate models was also evaluated via simulation; the OLS model performs significantly better than the Gaussian-Matérn model. PMID:26880257

  10. Measurement of changes in viscosity in polymers with gamma-ray dose using a differential viscometer

    NASA Astrophysics Data System (ADS)

    Santra, L.; Bhaumik, D.; Roy, S. C.

    1989-08-01

    Although some works on changes in viscosity of liquids with gamma-ray dose have been made near the "gel point", very little works have been done below this point. Changes in viscosities of different-grade silicone fluids below gel point have been measured using a differential viscometer developed in our laboratory, capable of measuring change in viscosities of two liquids directly. Preliminary results on viscosity changes when irradiated with energetic alpha particles will also be reported.

  11. NOTE: Total body-calcium measurements: comparison of two delayed-gamma neutron activation facilities

    NASA Astrophysics Data System (ADS)

    Ma, R.; Ellis, K. J.; Yasumura, S.; Shypailo, R. J.; Pierson, R. N., Jr.

    1999-06-01

    This study compares two independently calibrated delayed-gamma neutron activation (DGNA) facilities, one at the Brookhaven National Laboratory (BNL), Upton, New York, and the other at the Children's Nutrition Research Center (CNRC), Houston, Texas that measure total body calcium (TBCa). A set of BNL phantoms was sent to CNRC for neutron activation analysis, and a set of CNRC phantoms was measured at BNL. Both facilities showed high precision (<2%), and the results were in good agreement, within 5%.

  12. Gross Gamma Dose Rate Measurements for TRIGA Spent Nuclear Fuel Burnup Validation

    SciTech Connect

    Winston, Philip Lon; Sterbentz, James William

    2001-04-01

    Gross gamma-ray dose rates from six spent TRIGA fuel elements were measured and compared to calculated values as a means to validate the reported element burnups. A newly installed and functional gamma-ray detection subsystem of the In-Cell Examination System was used to perform the measurements and is described in some detail. The analytical methodology used to calculate the corresponding dose rates is presented along with the calculated values. Comparison of the measured and calculated dose rates for the TRIGA fuel elements indicates good agreement (less than a factor of 2 difference). The intent of the subsystem is to measure the gross gamma dose rate and correlate the measurement to a calculated dose rate based on the element s known burnup and other pertinent spent fuel information. Although validation of the TRIGA elements’ burnup is of primary concern in this paper, the measurement and calculational techniques can be used to either validate an element’s reported burnup or provide a burnup estimate for an element with an unknown burnup.

  13. Intercomparison of inductively coupled plasma mass spectrometry, quantitative neutron capture radiography, and prompt gamma activation analysis for the determination of boron in biological samples.

    PubMed

    Schütz, C L; Brochhausen, C; Hampel, G; Iffland, D; Kuczewski, B; Otto, G; Schmitz, T; Stieghorst, C; Kratz, J V

    2012-10-01

    Boron determination in blood and tissue samples is a crucial task especially for treatment planning, preclinical research, and clinical application of boron neutron capture therapy (BNCT). Comparison of clinical findings remains difficult due to a variety of analytical methods, protocols, and standard reference materials in use. This paper addresses the comparability of inductively coupled plasma mass spectrometry, quantitative neutron capture radiography, and prompt gamma activation analysis for the determination of boron in biological samples. It was possible to demonstrate that three different methods relying on three different principles of sample preparation and boron detection can be validated against each other and yield consistent results for both blood and tissue samples. The samples were obtained during a clinical study for the application of BNCT for liver malignancies and therefore represent a realistic situation for boron analysis.

  14. Analytical Validation of Accelerator Mass Spectrometry for Pharmaceutical Development: the Measurement of Carbon-14 Isotope Ratio.

    SciTech Connect

    Keck, B D; Ognibene, T; Vogel, J S

    2010-02-05

    Accelerator mass spectrometry (AMS) is an isotope based measurement technology that utilizes carbon-14 labeled compounds in the pharmaceutical development process to measure compounds at very low concentrations, empowers microdosing as an investigational tool, and extends the utility of {sup 14}C labeled compounds to dramatically lower levels. It is a form of isotope ratio mass spectrometry that can provide either measurements of total compound equivalents or, when coupled to separation technology such as chromatography, quantitation of specific compounds. The properties of AMS as a measurement technique are investigated here, and the parameters of method validation are shown. AMS, independent of any separation technique to which it may be coupled, is shown to be accurate, linear, precise, and robust. As the sensitivity and universality of AMS is constantly being explored and expanded, this work underpins many areas of pharmaceutical development including drug metabolism as well as absorption, distribution and excretion of pharmaceutical compounds as a fundamental step in drug development. The validation parameters for pharmaceutical analyses were examined for the accelerator mass spectrometry measurement of {sup 14}C/C ratio, independent of chemical separation procedures. The isotope ratio measurement was specific (owing to the {sup 14}C label), stable across samples storage conditions for at least one year, linear over 4 orders of magnitude with an analytical range from one tenth Modern to at least 2000 Modern (instrument specific). Further, accuracy was excellent between 1 and 3 percent while precision expressed as coefficient of variation is between 1 and 6% determined primarily by radiocarbon content and the time spent analyzing a sample. Sensitivity, expressed as LOD and LLOQ was 1 and 10 attomoles of carbon-14 (which can be expressed as compound equivalents) and for a typical small molecule labeled at 10% incorporated with {sup 14}C corresponds to 30 fg

  15. Total Measurement Uncertainty for the Plutonium Finishing Plant (PFP) Segmented Gamma Scan Assay System

    SciTech Connect

    WESTSIK, G.A.

    2001-06-06

    This report presents the results of an evaluation of the Total Measurement Uncertainty (TMU) for the Canberra manufactured Segmented Gamma Scanner Assay System (SGSAS) as employed at the Hanford Plutonium Finishing Plant (PFP). In this document, TMU embodies the combined uncertainties due to all of the individual random and systematic sources of measurement uncertainty. It includes uncertainties arising from corrections and factors applied to the analysis of transuranic waste to compensate for inhomogeneities and interferences from the waste matrix and radioactive components. These include uncertainty components for any assumptions contained in the calibration of the system or computation of the data. Uncertainties are propagated at 1 sigma. The final total measurement uncertainty value is reported at the 95% confidence level. The SGSAS is a gamma assay system that is used to assay plutonium and uranium waste. The SGSAS system can be used in a stand-alone mode to perform the NDA characterization of a container, particularly for low to medium density (0-2.5 g/cc) container matrices. The SGSAS system provides a full gamma characterization of the container content. This document is an edited version of the Rocky Flats TMU Report for the Can Scan Segment Gamma Scanners, which are in use for the plutonium residues projects at the Rocky Flats plant. The can scan segmented gamma scanners at Rocky Flats are the same design as the PFP SGSAS system and use the same software (with the exception of the plutonium isotopics software). Therefore, all performance characteristics are expected to be similar. Modifications in this document reflect minor differences in the system configuration, container packaging, calibration technique, etc. These results are supported by the Quality Assurance Objective (QAO) counts, safeguards test data, calibration data, etc. for the PFP SGSAS system. Other parts of the TMU analysis utilize various modeling techniques such as Monte Carlo N

  16. The use of an active coded aperture for improved directional measurements in high energy gamma-ray astronomy

    NASA Technical Reports Server (NTRS)

    Johansson, A.; Beron, B. L.; Campbell, L.; Eichler, R.; Hofstadter, R.; Hughes, E. B.; Wilson, S.; Gorodetsky, P.

    1980-01-01

    The coded aperture, a refinement of the scatter-hole camera, offers a method for the improved measurement of gamma-ray direction in gamma-ray astronomy. Two prototype coded apertures have been built and tested. The more recent of these has 128 active elements of the heavy scintillator BGO. Results of tests for gamma-rays in the range 50-500 MeV are reported and future application in space discussed.

  17. Measurement of the positron-electron reaction which produces a gamma ray pair in the region psi/3684/

    NASA Technical Reports Server (NTRS)

    Hughes, E. B.; Beron, B. L.; Carrington, R. L.; Ford, R. L.; Hofstadter, R.; Liberman, A. D.; Martin, T. W.; Oneill, L. H.; Simpson, J. W.; Hilger, E.

    1976-01-01

    An experiment was conducted to measure gamma ray pairs produced in the electron-positron reaction in the region of psi(3684) resonance. The apparatus consisted of two identical spectrometers mounted in a collinear configuration about the beam interaction region. Graphs are presented for the coplanarity angle between reconstructed gamma ray directions, for the scattering and energy deposition of gamma rays in the two crystals used, and for the observed rate of annihilation reactions as a function of center of mass energy.

  18. Integral measurements of neutron and gamma-ray leakage fluxes from the Little Boy replica

    SciTech Connect

    Muckenthaler, F.J.

    1984-03-01

    This report presents integral measurements of neutron and gamma-ray leakage fluxes from a critical mockup of the Hiroshima bomb Little Boy at Los Alamos National Laobratory with detector systems developed by Oak Ridge National Laboratory. Bonner ball detectors were used to map the neutron fluxes in the horizontal midplane at various distances from the mockup and for selected polar angles, keeping the source-detector separation constant. Gamma-ray energy deposition measurements were made with thermoluminescent detectors at several locations on the iron shell of the source mockup. The measurements were performed as part of a larger progam to provide benchmark data for testing the methods used to calculate the radiation released from the Little Boy bomb over Hiroshima. 3 references, 10 figures.

  19. Impact energy measurement in time-of-flight mass spectrometry with cryogenic microcalorimeters.

    PubMed

    Hilton, G C; Martinis, J M; Wollman, D A; Irwin, K D; Dulcie, L L; Gerber, D; Gillevet, P M; Twerenbold, D

    1998-02-12

    Time-of-flight mass spectrometry-most notably matrix-assisted laser-desorption-ionization time-of-flight (MALDI-TOF) spectrometry-is an important class of techniques for the study of proteins and other biomolecules. Although these techniques provide excellent performance for masses up to about 20,000 daltons, there has been limited success in achieving good mass resolution at higher masses. This is because the sensitivity of the microchannel plate (MCP) detectors used in most systems decreases rapidly with increasing particle mass, limiting the utility of MCP detectors for very large masses. It has recently been proposed that cryogenic particle detectors may provide a solution to these difficulties. Cryogenic detectors measure the thermal energy deposited by the particle impact, and thus have a sensitivity that is largely independent of particle mass. Recent experiments have demonstrated the sensitivity of cryogenic particle detectors to single biomolecules, a quantum efficiency several orders of magnitude larger than the MCP detectors, and sensitivity to masses as large as 750,000 daltons. Here we present results demonstrating an order of magnitude better energy resolution than previous measurements, allowing direct determination of particle charge state during acceleration. Although application of these detectors to practical mass spectrometry will require further development of the detectors and cryogenics, these detectors can be used to elucidate the performance-limiting processes that occur in such systems.

  20. A reanalysis of radioisotope measurements of the $^9$Be$$(\\gamma,n)^8$$Be cross-section

    DOE PAGES

    Robinson, Alan E.

    2016-02-18

    Themore » $^9$Be$$(\\gamma,n)^8$$Be reaction is enhanced by a near threshold $1/2^+$ state. Contradictions between existing measurements of this reaction cross-section affect calculations of astrophysical r-process yields, dark matter detector calibrations, and the theory of the nuclear structure of $^9$Be. Select well-documented radioisotope $^9$Be$$(\\gamma,n)$$ source yield measurements have been reanalyzed, providing a set of high-accuracy independently measured cross sections. A Breit-Wigner fit of these corrected measurements yields $$E_R=1738.8\\pm1.9$$ keV, $$\\Gamma_\\gamma=0.771\\pm0.021$$ eV, and $$\\Gamma_n=268\\pm15$$ keV for the $1/2^+$ state. A virtual $1/2^+$ state is excluded with 99.3\\% confidence.« less

  1. PING Gamma Ray and Neutron Measurements of a Meter-Sized Carbonaceous Asteroid Analog

    NASA Technical Reports Server (NTRS)

    Bodnarik, J.; Burger, D.; Evans, L.; Floyd, S.; Lim, L.; McClanahan, T.; Namkung, M.; Nowicki, S.; Parsons, A.; Schweitzer, J.; Starr, R.; Trombka, J.

    2011-01-01

    Determining the elemental composition of carbonaceous (spectral type C) asteroids is still one of the basic problems when studying these objects. The only main source of elemental composition information for asteroids is from their optical, NIR and IR properties, which include their spectral reflectance characteristics, albedo, polarization, and the comparison of optical spectroscopy with meteorite groups corresponding to asteroids of every spectral type. Unfortunately, these sources reflect observations from widely contrasting spatial scales that presently yield a void in the continuum of microscopic and macroscopic evidence, a lack of in situ measurement confirmation, and require deeper sensing techniques to discern the nature of these asteroids. The Probing In situ with Neutrons and Gamma rays (PING) instrument is ideally suited to address this problem because it can be used to determine the bulk elemental composition, H and C content, the average atomic weight and density of the surface and subsurface layers of C-type asteroids, and can provide measurements used to determine the difference between and distinguish between different types of asteroids. We are currently developing the PING instrument that combines gamma ray and neutron detectors with a 14 Me V pulsed neutron generator to determine the in-situ bulk elemental abundances and geochemistry of C-type asteroids with a spatial resolution of 1 m down to depths of tens of cm to 1 m. One aspect of the current work includes experimentally testing and optimizing PING on a known meter-sized Columbia River basalt C-type asteroid analog sample that has a similar composition and the same neutron response as that of a C-type asteroid. An important part of this effort focuses on utilizing timing measurements to isolate gamma rays produced by neutron inelastic scattering, neutron capture and delayed activation processes. Separating the gamma ray spectra by nuclear processes results in higher precision and sensitivity

  2. Improving precision in resonance ionization mass spectrometry : influence of laser bandwidth in uranium isotope ratio measurements.

    SciTech Connect

    Isselhardt, B. H.; Savina, M. R.; Knight, K. B.; Pellin, M. J.; Hutcheon, I. D.; Prussin, S. G.

    2011-03-01

    The use of broad bandwidth lasers with automated feedback control of wavelength was applied to the measurement of {sup 235}U/{sup 238}U ratios by resonance ionization mass spectrometry (RIMS) to decrease laser-induced isotopic fractionation. By broadening the bandwidth of the first laser in a three-color, three-photon ionization process from a bandwidth of 1.8 GHz to about 10 GHz, the variation in sequential relative isotope abundance measurements decreased from 10% to less than 0.5%. This procedure was demonstrated for the direct interrogation of uranium oxide targets with essentially no sample preparation.

  3. Radionuclides in man and his environment measured by accelerator mass spectrometry

    SciTech Connect

    Hellborg, Ragnar; Erlandsson, Bengt; Kiisk, Madis; Persson, Per; Skog, Goeran; Stenstroem, Kristina; Mattsson, Soeren; Leide-Svegborn, Sigrid; Olofsson, Mikael

    1999-06-10

    Accelerator mass spectrometry (AMS) is a highly sensitive analytical method for measuring very low concentrations of both radionuclides and stable nuclides. For radioanalytical purposes, the main advantages of AMS compared to conventional radiometric methods are the use of smaller samples (mg size) and shorter measuring times (less than one hour). In this report some current applications of the AMS technique at the Lund Pelletron accelerator are presented, in particular studies of {sup 14}C-labeled pharmaceuticals used in clinical nuclear medicine and biomedical research.

  4. PC/FRAM: Algorithms for the gamma-ray spectrometry measurement of plutonium isotopic composition

    SciTech Connect

    Kelley, T.A.; Sampson, T.E.; DeLapp, D.

    1995-10-01

    The Safeguards Program at Los Alamos National Laboratory has developed versatile software for the isotopic analysis of SNM in a sample. The FRAM code has been used routinely at LANL for years. Its capability has now been greatly expanded, and it has been given a graphical user interface. Some of the details on the internal workings of the code are given in this paper.

  5. Comparison of electrical capacitance tomography & gamma densitometer measurement in viscous oil-gas flows

    NASA Astrophysics Data System (ADS)

    Archibong Eso, A.; Zhao, Yabin; Yeung, Hoi

    2014-04-01

    Multiphase flow is a common occurrence in industries such as nuclear, process, oil & gas, food and chemical. A prior knowledge of its features and characteristics is essential in the design, control and management of such processes due to its complex nature. Electrical Capacitance Tomography (ECT) and Gamma Densitometer (Gamma) are two promising approaches for multiphase visualization and characterization in process industries. In two phase oil & gas flow, ECT and Gamma are used in multiphase flow monitoring techniques due to their inherent simplicity, robustness, and an ability to withstand wide range of operational temperatures and pressures. High viscous oil (viscosity > 100 cP) is of interest because of its huge reserves, technological advances in its production and unlike conventional oil (oil viscosity < 100 cP) and gas flows where ECT and Gamma have been previously used, high viscous oil and gas flows comes with certain associated concerns which include; increased entrainment of gas bubbles dispersed in oil, shorter and more frequent slugs as well as oil film coatings on the walls of flowing conduits. This study aims to determine the suitability of both devices in the visualization and characterization of high-viscous oil and gas flow. Static tests are performed with both devices and liquid holdup measurements are obtained. Dynamic experiments were also conducted in a 1 & 3 inch facility at Cranfield University with a range of nominal viscosities (1000, 3000 & 7500 cP). Plug, slug and wavy annular flow patterns were identified by means of Probability Mass Function and time series analysis of the data acquired from Gamma and ECT devices with high speed camera used to validate the results. Measured Liquid holdups for both devices were also compared.

  6. Comparison of electrical capacitance tomography and gamma densitometer measurement in viscous oil-gas flows

    SciTech Connect

    Archibong Eso, A.; Zhao, Yabin; Yeung, Hoi

    2014-04-11

    Multiphase flow is a common occurrence in industries such as nuclear, process, oil and gas, food and chemical. A prior knowledge of its features and characteristics is essential in the design, control and management of such processes due to its complex nature. Electrical Capacitance Tomography (ECT) and Gamma Densitometer (Gamma) are two promising approaches for multiphase visualization and characterization in process industries. In two phase oil and gas flow, ECT and Gamma are used in multiphase flow monitoring techniques due to their inherent simplicity, robustness, and an ability to withstand wide range of operational temperatures and pressures. High viscous oil (viscosity > 100 cP) is of interest because of its huge reserves, technological advances in its production and unlike conventional oil (oil viscosity < 100 cP) and gas flows where ECT and Gamma have been previously used, high viscous oil and gas flows comes with certain associated concerns which include; increased entrainment of gas bubbles dispersed in oil, shorter and more frequent slugs as well as oil film coatings on the walls of flowing conduits. This study aims to determine the suitability of both devices in the visualization and characterization of high-viscous oil and gas flow. Static tests are performed with both devices and liquid holdup measurements are obtained. Dynamic experiments were also conducted in a 1 and 3 inch facility at Cranfield University with a range of nominal viscosities (1000, 3000 and 7500 cP). Plug, slug and wavy annular flow patterns were identified by means of Probability Mass Function and time series analysis of the data acquired from Gamma and ECT devices with high speed camera used to validate the results. Measured Liquid holdups for both devices were also compared.

  7. Results of Gamma-Ray Measurements from a Recent Demonstration for Russian Technical Experts

    SciTech Connect

    Luke, S J; Archer, D E; Gosnell, T B; Lochner, R T; Morgan, J F; White, G K; Weitz, R

    2001-06-01

    In August 2001, a group of U.S. technical experts demonstrated an Attribute Measurement System with an Information Barrier (AMSIB) for a delegation of Russian technical experts. The purpose of the demonstration was to show that attributes of a classified plutonium item of potential interest to arms control and nonproliferation transparency regimes could be ascertained without releasing any sensitive information. For this demonstration, both gamma-ray and neutron attributes were determined. We consider only the gamma-ray attributes here. The specific plutonium attributes measured were the isotopic ratio of {sup 240}Pu to {sup 239}Pu, the ''age'' of the plutonium (time elapsed since the most recent chemical purification of the plutonium), and the absence of plutonium oxide in the item's storage container. In this paper, we briefly review the technologies employed for the attribute measurements used in the gamma-ray portion of the demonstration, concentrating on the results of the test measurements of the isotopic and age attributes made on unclassified items.

  8. Fermi Large Area Telescope Measurements of the Diffuse Gamma-Ray Emission at Intermediate Galactic Latitudes

    NASA Astrophysics Data System (ADS)

    Abdo, A. A.; Ackermann, M.; Ajello, M.; Anderson, B.; Atwood, W. B.; Axelsson, M.; Baldini, L.; Ballet, J.; Barbiellini, G.; Bastieri, D.; Baughman, B. M.; Bechtol, K.; Bellazzini, R.; Berenji, B.; Blandford, R. D.; Bloom, E. D.; Bonamente, E.; Borgland, A. W.; Bregeon, J.; Brez, A.; Brigida, M.; Bruel, P.; Burnett, T. H.; Caliandro, G. A.; Cameron, R. A.; Caraveo, P. A.; Casandjian, J. M.; Cecchi, C.; Charles, E.; Chekhtman, A.; Cheung, C. C.; Chiang, J.; Ciprini, S.; Claus, R.; Cohen-Tanugi, J.; Conrad, J.; Dereli, H.; Dermer, C. D.; de Angelis, A.; de Palma, F.; Digel, S. W.; di Bernardo, G.; Dormody, M.; Do Couto E Silva, E.; Drell, P. S.; Dubois, R.; Dumora, D.; Edmonds, Y.; Farnier, C.; Favuzzi, C.; Fegan, S. J.; Focke, W. B.; Frailis, M.; Fukazawa, Y.; Funk, S.; Fusco, P.; Gaggero, D.; Gargano, F.; Gehrels, N.; Germani, S.; Giebels, B.; Giglietto, N.; Giordano, F.; Glanzman, T.; Godfrey, G.; Grenier, I. A.; Grondin, M.-H.; Grove, J. E.; Guillemot, L.; Guiriec, S.; Hanabata, Y.; Harding, A. K.; Hayashida, M.; Hays, E.; Hughes, R. E.; Jóhannesson, G.; Johnson, A. S.; Johnson, R. P.; Johnson, T. J.; Johnson, W. N.; Kamae, T.; Katagiri, H.; Kataoka, J.; Kawai, N.; Kerr, M.; Knödlseder, J.; Kocian, M. L.; Kuehn, F.; Kuss, M.; Lande, J.; Latronico, L.; Longo, F.; Loparco, F.; Lott, B.; Lovellette, M. N.; Lubrano, P.; Madejski, G. M.; Makeev, A.; Mazziotta, M. N.; McConville, W.; McEnery, J. E.; Meurer, C.; Michelson, P. F.; Mitthumsiri, W.; Mizuno, T.; Moiseev, A. A.; Monte, C.; Monzani, M. E.; Morselli, A.; Moskalenko, I. V.; Murgia, S.; Nolan, P. L.; Nuss, E.; Ohsugi, T.; Okumura, A.; Omodei, N.; Orlando, E.; Ormes, J. F.; Paneque, D.; Panetta, J. H.; Parent, D.; Pelassa, V.; Pepe, M.; Pesce-Rollins, M.; Piron, F.; Porter, T. A.; Rainò, S.; Rando, R.; Razzano, M.; Reimer, A.; Reimer, O.; Reposeur, T.; Ritz, S.; Rodriguez, A. Y.; Roth, M.; Ryde, F.; Sadrozinski, H. F.-W.; Sanchez, D.; Sander, A.; Saz Parkinson, P. M.; Scargle, J. D.; Sellerholm, A.; Sgrò, C.; Smith, D. A.; Smith, P. D.; Spandre, G.; Spinelli, P.; Starck, J.-L.; Stecker, F. W.; Striani, E.; Strickman, M. S.; Strong, A. W.; Suson, D. J.; Tajima, H.; Takahashi, H.; Tanaka, T.; Thayer, J. B.; Thayer, J. G.; Thompson, D. J.; Tibaldo, L.; Torres, D. F.; Tosti, G.; Tramacere, A.; Uchiyama, Y.; Usher, T. L.; Vasileiou, V.; Vilchez, N.; Vitale, V.; Waite, A. P.; Wang, P.; Winer, B. L.; Wood, K. S.; Ylinen, T.; Ziegler, M.

    2009-12-01

    The diffuse galactic γ-ray emission is produced by cosmic rays (CRs) interacting with the interstellar gas and radiation field. Measurements by the Energetic Gamma-Ray Experiment Telescope (EGRET) instrument on the Compton Gamma-Ray Observatory indicated excess γ-ray emission ≳1GeV relative to diffuse galactic γ-ray emission models consistent with directly measured CR spectra (the so-called “EGRET GeV excess”). The Large Area Telescope (LAT) instrument on the Fermi Gamma-Ray Space Telescope has measured the diffuse γ-ray emission with improved sensitivity and resolution compared to EGRET. We report on LAT measurements for energies 100 MeV to 10 GeV and galactic latitudes 10°≤|b|≤20°. The LAT spectrum for this region of the sky is well reproduced by a diffuse galactic γ-ray emission model that is consistent with local CR spectra and inconsistent with the EGRET GeV excess.

  9. Analyses of uranium and actinium gamma spectra: an application to measurements of environmental contamination

    SciTech Connect

    Momeni, M.H.

    1981-01-01

    A system for the reduction of the complex gamma spectra of nuclides in the uranium, actinium, and thorium series, tailored to calculation of line intensities, analyses of errors, and identification of nuclides is described. This system provides an efficient technique for characterizing contamination in the environs of uranium mines and mills. Identification of the nuclides and calculation of their concentrations require accurate knowledge of gamma energies and absolute quantum intensities. For some spectral lines, there are no reported measurements of absolute quantum intensities and in some cases where reports are available the measured intensities are not in agreement. In order to improve this data base, the spectra of gamma rays (of nuclides in the uranium and actinium series) with energies between 40 and 1400 keV were measured using high-resolution germanium detectors. A brief description of the spectroscopy system, computational algorithms for deconvolution, and methods of calibration for energy and efficiency, are described. The measured energies and absolute quantum intensities are compared with those reported in the literature.

  10. Measuring Thermodynamic Properties of Metals and Alloys With Knudsen Effusion Mass Spectrometry

    NASA Technical Reports Server (NTRS)

    Copland, Evan H.; Jacobson, Nathan S.

    2010-01-01

    This report reviews Knudsen effusion mass spectrometry (KEMS) as it relates to thermodynamic measurements of metals and alloys. First, general aspects are reviewed, with emphasis on the Knudsen-cell vapor source and molecular beam formation, and mass spectrometry issues germane to this type of instrument are discussed briefly. The relationship between the vapor pressure inside the effusion cell and the measured ion intensity is the key to KEMS and is derived in detail. Then common methods used to determine thermodynamic quantities with KEMS are discussed. Enthalpies of vaporization, the fundamental measurement, are determined from the variation of relative partial pressure with temperature using the second-law method or by calculating a free energy of formation and subtracting the entropy contribution using the third-law method. For single-cell KEMS instruments, measurements can be used to determine the partial Gibbs free energy if the sensitivity factor remains constant over multiple experiments. The ion-current ratio method and dimer-monomer method are also viable in some systems. For a multiple-cell KEMS instrument, activities are obtained by direct comparison with a suitable component reference state or a secondary standard. Internal checks for correct instrument operation and general procedural guidelines also are discussed. Finally, general comments are made about future directions in measuring alloy thermodynamics with KEMS.

  11. Safeguards Verification Measurements using Laser Ablation, Absorbance Ratio Spectrometry in Gaseous Centrifuge Enrichment Plants

    SciTech Connect

    Anheier, Norman C.; Cannon, Bret D.; Kulkarni, Gourihar R.; Munley, John T.; Nelson, Danny A.; Qiao, Hong; Phillips, Jon R.

    2012-07-17

    Laser Ablation Absorbance Ratio Spectrometry (LAARS) is a new verification measurement technology under development at the US Department of Energy (DOE) Pacific Northwest National Laboratory (PNNL). LAARS uses three lasers to ablate and then measure the relative isotopic abundance of uranium compounds. An ablation laser is tightly focused on uranium-bearing solids, producing a small atomic uranium vapor plume. Two collinear wavelength-tuned spectrometry lasers transit through the plume and the absorbance of U-235 and U-238 isotopes are measured to determine U-235 enrichment. The measurement is independent of chemical form and degree of dilution with nuisance dust and other materials. LAARS has high relative precision and detection limits approaching the femtogram range for U-235. The sample is scanned and assayed point-by-point at rates reaching 1 million measurements/hour, enabling LAARS to detect and analyze uranium in trace samples. The spectrometer is assembled using primarily commercially available components and features a compact design and automated analysis.Two specific gaseous centrifuge enrichment plant (GCEP) applications of the spectrometer are currently under development: 1) LAARS-Environmental Sampling (ES), which collects and analyzes aerosol particles for GCEP misuse detection and 2) LAARS-Destructive Assay (DA), which enables onsite enrichment DA sample collection and analysis for protracted diversion detection. The two applications propose game-changing technological advances in GCEP safeguards verification.

  12. Measurement of gamma + c + X and gamma + b + X production cross sections at s**(1/2) = 1.96-TeV

    SciTech Connect

    Duggan, Daniel; /Florida State U.

    2009-06-01

    The photon plus heavy-flavour quark (b, c) final state provides a unique and valuable window into both the sea quark content of the proton and the splitting of gluons into heavy-flavour quark pairs. A new combination of experimental techniques has provided the basis for the first measurements of the differential {gamma} + c + X and {gamma} + b + X production cross sections at {radical}s = 1.96 TeV. The measurements use {approx} 1 fb{sup -1} of data from p{bar p} collisions collected with the D0 detector.

  13. High resolution gamma ray tomography scanner for flow measurement and non-destructive testing applications

    NASA Astrophysics Data System (ADS)

    Hampel, U.; Bieberle, A.; Hoppe, D.; Kronenberg, J.; Schleicher, E.; Sühnel, T.; Zimmermann, F.; Zippe, C.

    2007-10-01

    We report on the development of a high resolution gamma ray tomography scanner that is operated with a Cs-137 isotopic source at 662keV gamma photon energy and achieves a spatial image resolution of 0.2linepairs/mm at 10% modulation transfer function for noncollimated detectors. It is primarily intended for the scientific study of flow regimes and phase fraction distributions in fuel element assemblies, chemical reactors, pipelines, and hydrodynamic machines. Furthermore, it is applicable to nondestructive testing of larger radiologically dense objects. The radiation detector is based on advanced avalanche photodiode technology in conjunction with lutetium yttrium orthosilicate scintillation crystals. The detector arc comprises 320 single detector elements which are operated in pulse counting mode. For measurements at fixed vessels or plant components, we built a computed tomography scanner gantry that comprises rotational and translational stages, power supply via slip rings, and data communication to the measurement personal computer via wireless local area network.

  14. Measurement of the 60Fe(n, gamma)61Fe Cross Section at Stellar Temperatures.

    PubMed

    Uberseder, E; Reifarth, R; Schumann, D; Dillmann, I; Pardo, C Domingo; Görres, J; Heil, M; Käppeler, F; Marganiec, J; Neuhausen, J; Pignatari, M; Voss, F; Walter, S; Wiescher, M

    2009-04-17

    Observations of galactic gamma-ray activity have challenged the current understanding of nucleosynthesis in massive stars. Recent measurements of (60)Fe abundances relative to ;{26}Al;{g} have underscored the need for accurate nuclear information concerning the stellar production of (60)Fe. In light of this motivation, a first measurement of the stellar (60)Fe(n, gamma)(61)Fe cross section, the predominant destruction mechanism of (60)Fe, has been performed by activation at the Karlsruhe Van de Graaff accelerator. Results show a Maxwellian averaged cross section at kT = 25 keV of 9.9 +/-_{1.4(stat)};{2.8(syst)}mbarn, a significant reduction in uncertainty with respect to existing theoretical discrepancies. This result will serve to significantly constrain models of (60)Fe nucleosynthesis in massive stars. PMID:19518614

  15. Exclusive Measurements of the b to s gamma Transition Rate and Photon Energy Spectrum

    SciTech Connect

    Lees, J.P.; Poireau, V.; Tisserand, V.; Garra Tico, J.; Grauges, E.; Palano, A.; Eigen, G.; Stugu, B.; Brown, David Nathan; Kerth, L.T.; Kolomensky, Yu.G.; Lynch, G.; Koch, H.; Schroeder, T.; Asgeirsson, D.J.; Hearty, C.; Mattison, T.S.; McKenna, J.A.; Khan, A.; Blinov, V.E.; Buzykaev, A.R.; /more authors..

    2012-08-30

    We use 429 fb{sup -1} of e{sup +}e{sup -} collision data collected at the {Upsilon}(4S) resonance with the BABAR detector to measure the radiative transition rate of b {yields} s{gamma} with a sum of 38 exclusive final states. The inclusive branching fraction with a minimum photon energy of 1.9 GeV is found to be {Beta}({bar B} {yields} Xs{gamma}) = (3.29 {+-} 0.19 {+-} 0.48) x 10{sup -4} where the first uncertainty is statistical and the second is systematic. We also measure the first and second moments of the photon energy spectrum and extract the best fit values for the heavy-quark parameters, m{sub b} and {mu}{sub {pi}}{sup 2}, in the kinetic and shape function models.

  16. An industrial radiography exposure device based on measurement of transmitted gamma-ray intensity

    NASA Astrophysics Data System (ADS)

    Polee, C.; Chankow, N.; Srisatit, S.; Thong-Aram, D.

    2015-05-01

    In film radiography, underexposure and overexposure may happen particularly when lacking information of specimen material and hollowness. This paper describes a method and a device for determining exposure in industrial gamma-ray radiography based on quick measurement of transmitted gamma-ray intensity with a small detector. Application software was developed for Android mobile phone to remotely control the device and to display counting data via Bluetooth communication. Prior to film exposure, the device is placed behind a specimen to measure transmitted intensity which is inversely proportional to the exposure. Unlike in using the conventional exposure curve, correction factors for source decay, source-to- film distance, specimen thickness and kind of material are not needed. The developed technique and device make radiographic process economic, convenient and more reliable.

  17. Gamma ray facilities at the University of Maryland cyclotron. [data acquisition and radiation measurement

    NASA Technical Reports Server (NTRS)

    Hornyak, W. F.

    1978-01-01

    A special beam line was set up in a separate shielded experimental room to provide a low background station for gamma-ray measurements at the University of Maryland cyclotron. The transmitted beam leaving the target is gathered in by a magnetic quadrupole lens located 1.8 m further downstream and focused on a Faraday cup located on the far side of the 2.5 m thick concrete shielding wall of the experimental room. A software computer program permits timing information ot be obtained using the cyclotron beam fine structure as a time reference for the observed gamma-ray events. Measurements indicate a beam fine structure width of less than 1.2 nanoseconds repeated, for example, in the case of 140 MeV alpha particles every 90 nanoseconds. Twelve contiguous time channels of adjustable width may be set as desired with reference to the RF signal. This allows the creation of 12 separate 8192 channel analyzers.

  18. Improved Gamma Bang Time Measurements on Omega and Implications for the National Ignition Facility

    SciTech Connect

    Edward K. Miller , H. W. Hermann, S. E. Caldwell, S. C. Evans, J. M. Mack, P. Shanch, T. Sedillo, C. S. Young; C. J. Holrsfield, D. Drew; V. Yu Glebov

    2007-09-14

    The time of peak fusion reactivity with respect to the impingement of laser light on an ICF capsule is known as Bang Time (BT). This is an essential parameter in the understanding of ICF implosions. Traditionally, BT has been determined through temporal measurements of 14 MeV fusion neutrons. Because the neutron energy spectrum is Doppler broadened, the detector must be positioned close to target-chamber center in order to minimize the neutron temporal spreading which can compromise such a measurement. Fusion gammas, on the other hand, are not subject to temporal spreading, making proximity of the detector to the source a lesser concern. However, the low branching ratio for DT fusion reactions producing gammas ({approx}1e-4) presents detector sensitivity challenges.

  19. High resolution gamma ray tomography scanner for flow measurement and non-destructive testing applications

    SciTech Connect

    Hampel, U.; Bieberle, A.; Hoppe, D.; Kronenberg, J.; Schleicher, E.; Suehnel, T.; Zimmermann, F.; Zippe, C.

    2007-10-15

    We report on the development of a high resolution gamma ray tomography scanner that is operated with a Cs-137 isotopic source at 662 keV gamma photon energy and achieves a spatial image resolution of 0.2 line pairs/mm at 10% modulation transfer function for noncollimated detectors. It is primarily intended for the scientific study of flow regimes and phase fraction distributions in fuel element assemblies, chemical reactors, pipelines, and hydrodynamic machines. Furthermore, it is applicable to nondestructive testing of larger radiologically dense objects. The radiation detector is based on advanced avalanche photodiode technology in conjunction with lutetium yttrium orthosilicate scintillation crystals. The detector arc comprises 320 single detector elements which are operated in pulse counting mode. For measurements at fixed vessels or plant components, we built a computed tomography scanner gantry that comprises rotational and translational stages, power supply via slip rings, and data communication to the measurement personal computer via wireless local area network.

  20. Measurement of DT fusion and neutron-induced gamma-rays using gas Cherenkov Detector

    NASA Astrophysics Data System (ADS)

    Kim, Y.; Herrmann, H. W.; Evans, S.; Sedillo, T.; Langenbrunner, J. R.; Young, C. S.; Mack, J. M.; McEvoy, A.; Horsfield, C. J.; Rubery, M.; Ali, Z.; Stoeffl, W.

    2010-08-01

    A secondary gamma experiment was carried out using a Gas Cherenkov Detector (GCD) at the OMEGA laser facility. The primary experimental objective was to simulate neutron-induced secondary gamma production (n-γ) from a NIF implosion capsule, hohlraum, and thermo-mechanical package. The high-band width of the GCD enabled us to detect time delayed and Doppler broadened n-γ signals from five different puck materials (Si, SiO2, Al, Al2O3, Cu) placed near target chamber center. These measurements were used for MCNP & ITS ACCEPT code validation purposes. By a simple change of the GCD CO2 gas pressure the system can effectively eliminate signals induced by n-γ reactions and thereby allow quality measurements of DT fusion γ-rays that are produced at NIF (National Ignition Facility).

  1. Multipurpose Radiation Resistant Semiconductor Detectors for Alpha, Neutron & Low Energy Gamma Ray Measurements at High Temperatures in High-Intensity Gamma Ray

    SciTech Connect

    Ruddy, Frank H.

    2005-06-01

    Work scheduled under year two of DOE Grant DE-FG02-04ER63734 is on schedule and all year-two milestones have or will be met. Results to date demonstrate that unprecedented silicon carbide (SiC) energy resolution has been obtained, and that SiC detectors may achieve energy resolution that exceeds that obtainable with the best silicon alpha spectrometers. Fast-neutron energy spectrometry measurements indicate that recoil-ion energy spectrometry should be possible with SiC detectors. Furthermore, SiC detectors have been demonstrated to perform well even after gamma-ray exposures of 1.E09 Rad. This result and the previously demonstrated capability of SiC detectors to operate in elevated-temperature environments are very promising for potential DOE EMSP applications. A new class of multipurpose, radiation-resistant semiconductor detectors that can be used in elevated-temperature and high-radiation environments is being developed under this grant. These detectors, based on silicon carbide (SiC) semiconductor are designed to have larger active volumes than previously available SiC detectors, and are being tested for their response to alpha particles, X-rays and low energy gamma rays, and fast neutrons. Specifically, SiC radiation detectors with larger areas and 100-micrometer thick active regions have been designed and manufactured according to detector-design specifications. Detectors based on a Schottky diode design were specified in order to minimize the effects of the detector entrance window on alpha particle measurements. During manufacture of the Schottky diodes, the manufacturer also provided a set of large-volume SiC p-i-n diodes for testing Extensive alpha particle measurements have been carried out to test and quantify the response of the SiC Schottky diodes. Exposures to 148-Gd, 213-Po, 217-At, 221-Fr, 225-Ac, 237-Np, 238-Pu, 240-Pu, and 242-Pu sources were used to obtain detailed alpha response data in the alpha energy range from 3182.787 keV to 8375.9 ke

  2. Technical Note: PRESAGE three-dimensional dosimetry accurately measures Gamma Knife output factors

    PubMed Central

    Klawikowski, Slade J.; Yang, James N.; Adamovics, John; Ibbott, Geoffrey S.

    2014-01-01

    Small-field output factor measurements are traditionally very difficult because of steep dose gradients, loss of lateral electronic equilibrium, and dose volume averaging in finitely sized detectors. Three-dimensional (3D) dosimetry is ideal for measuring small output factors and avoids many of these potential challenges of point and two-dimensional detectors. PRESAGE 3D polymer dosimeters were used to measure the output factors for the 4 mm and 8 mm collimators of the Leksell Perfexion Gamma Knife radiosurgery treatment system. Discrepancies between the planned and measured distance between shot centers were also investigated. A Gamma Knife head frame was mounted onto an anthropomorphic head phantom. Special inserts were machined to hold 60 mm diameter, 70 mm tall cylindrical PRESAGE dosimeters. The phantom was irradiated with one 16 mm shot and either one 4 mm or one 8 mm shot, to a prescribed dose of either 3 Gy or 4 Gy to the 50% isodose line. The two shots were spaced between 30 mm and 60 mm apart and aligned along the central axis of the cylinder. The Presage dosimeters were measured using the DMOS-RPC optical CT scanning system. Five independent 4 mm output factor measurements fell within 2% of the manufacturer’s Monte Carlo simulation-derived nominal value, as did two independent 8 mm output factor measurements. The measured distances between shot centers varied by ± 0.8 mm with respect to the planned shot displacements. On the basis of these results, we conclude that PRESAGE dosimetry is excellently suited to quantify the difficult-to-measure Gamma Knife output factors. PMID:25368961

  3. Time-resolved inductively coupled plasma mass spectrometry measurements with individual, monodisperse drop sample introduction.

    PubMed

    Dziewatkoski, M P; Daniels, L B; Olesik, J W

    1996-04-01

    Individual ion clouds, each produced in the ICP from a single drop of sample, were monitored using time-resolved mass spectrometry and optical emission spectrometry simultaneously. The widths of the ion clouds in the plasma as a function of distance from the point of initial desolvated particle vaporization in the ICP were estimated. The Li(+) cloud width (full width at halfmaximum) varied from 85 to 272 μs at 3 and 10 mm from the apparent vaporization point, respectively. The Sr(+) cloud width varied from 97 to 142 μs at 5 and 10 mm from the apparent vaporization point, respectively. The delays between optical and mass spectrometry signals were used to measure gas velocities in the ICP. The velocity data could then be used to convert ion cloud peak widths in time to cloud sizes in the ICP. Li(+) clouds varied from 2.1 to 6.6 mm (full width at half-maximum) and Sr(+) clouds varied from 2.4 to 3.5 mm at the locations specified above. Diffusion coefficients were estimated from experimental data to be 88, 44, and 24 cm(2)/s for Li(+), Mg(+), and Sr(+), respectively. The flight time of ions from the sampling orifice of the mass spectrometer to the detector were mass dependent and varied from 13 to 21 μs for Mg(+) to 93 to 115 μs for Pb(+).

  4. Unveiling the Nature of Soft Gamma Repeaters and Magnetars: Scientists Measure the Most Powerful Magnet Known

    NASA Technical Reports Server (NTRS)

    Swank, Jean (Technical Monitor); Parke, William

    2002-01-01

    This newsletter from NASA Goddard Space Flight Center (GSFC) announces measurements of the magnetic field of a magnetar. The magnetic field was approx. 10(exp 15) gauss, up to 10 times more powerful than previous estimates. The newsletter also describes how the star's magnetic field slows its rotation, and how starquakes emit protons, which are trapped in this neutron star's magnetic field, and make it a soft gamma repeater (SGR).

  5. Borehole field calibration and measurement of low-concentration manganese by decay gamma rays ( Maryland, USA).

    USGS Publications Warehouse

    Mikesell, J.L.; Senftle, F.E.; Lloyd, T.A.; Tanner, A.B.; Merritt, C.T.; Force, E.R.

    1986-01-01

    The Mn concentration in the Arundel clay formation, Prince Georges County, Maryland, was determined from a borehole by using delayed neutron activation. Then neutrons were produced by a 100 mu g 252Cf source. The 847 keV gamma ray of Mn was detected continuously, and its counting rate was measured at intervals of 15 s as the measuring sonde was moved at a rate of 0.5 cm/s. The borehole measurements compared favourably with a chemical core analysis and were unaffected by water in the borehole.-from Authors

  6. Safeguards Verification Measurements using Laser Ablation, Absorbance Ratio Spectrometry in Gaseous Centrifuge Enrichment Plants

    SciTech Connect

    Anheier, Norman C.; Cannon, Bret D.; Qiao, Hong; Phillips, Jon R.

    2012-07-01

    Laser Ablation Absorbance Ratio Spectrometry (LAARS) is a new verification measurement technology under development at the US Department of Energy’s (DOE) Pacific Northwest National Laboratory (PNNL). LAARS uses three lasers to ablate and then measure the relative isotopic abundance of uranium compounds. An ablation laser is tightly focused on uranium-bearing solids producing a small plume containing uranium atoms. Two collinear wavelength-tuned spectrometry lasers transit through the plume and the absorbance of U-235 and U-238 isotopes are measured to determine U-235 enrichment. The measurement has high relative precision and detection limits approaching the femtogram range for uranium. It is independent of chemical form and degree of dilution with nuisance dust and other materials. High speed sample scanning and pinpoint characterization allow measurements on millions of particles/hour to detect and analyze the enrichment of trace uranium in samples. The spectrometer is assembled using commercially available components at comparatively low cost, and features a compact and low power design. Future designs can be engineered for reliable, autonomous deployment within an industrial plant environment. Two specific applications of the spectrometer are under development: 1) automated unattended aerosol sampling and analysis and 2) on-site small sample destructive assay measurement. The two applications propose game-changing technological advances in gaseous centrifuge enrichment plant (GCEP) safeguards verification. The aerosol measurement instrument, LAARS-environmental sampling (ES), collects aerosol particles from the plant environment in a purpose-built rotating drum impactor and then uses LAARS-ES to quickly scan the surface of the impactor to measure the enrichments of the captured particles. The current approach to plant misuse detection involves swipe sampling and offsite analysis. Though this approach is very robust it generally requires several months to

  7. Gamma radiation measurements and dose rates in commercially-used natural tiling rocks (granites).

    PubMed

    Tzortzis, Michalis; Tsertos, Haralabos; Christofides, Stelios; Christodoulides, George

    2003-01-01

    The gamma radiation in samples of a variety of natural tiling rocks (granites) imported in Cyprus for use in the building industry was measured, employing high-resolution gamma-ray spectroscopy. The rock samples were pulverised, sealed in 1-l plastic Marinelli beakers, and measured in the laboratory with an accumulating time between 10 and 14 h each. From the measured gamma-ray spectra, activity concentrations were determined for (232)Th (range from 1 to 906 Bq kg(-1)), (238)U (from 1 to 588 Bq kg(-1)) and (40)K (from 50 to 1606 Bq kg(-1)). The total absorbed dose rates in air calculated from the concentrations of the three radionuclides ranged from 7 to 1209 nGy h(-1) for full utilization of the materials, from 4 to 605 nGy h(-1) for half utilization and from 2 to 302 nGy h(-1) for one quarter utilization. The total effective dose rates per person indoors were determined to be between 0.02 and 2.97 mSv y(-1) for half utilization of the materials. Applying dose criteria recently recommended by the EU for superficial materials, 25 of the samples meet the exemption dose limit of 0.3 mSv y(-1), two of them meet the upper dose limit of 1 mSv y(-1) and only one clearly exceeds this limit.

  8. Global Elemental Maps of the Moon Using Gamma Rays Measured by the Kaguya (SELENE) Mission

    NASA Astrophysics Data System (ADS)

    Reedy, Robert C.; Hasebe, N.; Yamashita, N.; Karouji, Y.; Kobayashi, S.; Hareyama, M.; Hayatsu, K.; Okudaira, O.; Kobayashi, M.; d'Uston, C.; Maurice, S.; Gasnault, O.; Forni, O.; Diez, B.; Kim, K.

    2009-09-01

    The Kaguya spacecraft was in a circular polar lunar orbit from 17 October 2007 until 10 June 2009 as part of JAXA's SELENE lunar exploration program. Among the 13 instruments, an advanced gamma-ray spectrometer (GRS) studied the distributions of many elements. The gamma rays were from the decay of the naturally-radioactive elements K, Th, and U and from cosmic-ray interactions with H, O, Mg, Al, Si, Ca, Ti, Fe, and other elements. They are emitted from the top few tens of centimeters of the lunar surface. The main detector of the GRS was high-purity germanium, which was surrounded by bismuth germanate and plastic scintillators to reduce backgrounds. Gamma-ray spectra were sent to the Earth every 17 seconds (1 degree of the lunar surface) with energies from 0-12 MeV. These spectra were adjusted to a standard gain and then summed over many lunar regions. Background spectra were also determined. Over 200 gamma rays have been observed, with most being backgrounds but many being from the lunar surface, an order more gamma rays than from any previous lunar GRS missions. Elemental results have been determined for K, Th, and U. Results for K and Th are consistent with those from the GRS on Apollo and Lunar Prospector. The first lunar global maps for U have been determined. These 3 elements show strong correlations among themselves, which implies that the Moon is homogeneous in these elements over the entire Moon. Their elemental ratios agree well with those measured in lunar samples and meteorites. Preliminary maps for Fe are consistent with earlier maps. Other elements, including O, Mg, Si, Ca, and Ti, are being mapped, and their distributions vary over the lunar surface and appear consistent with previous lunar elemental results. This work was supported by JAXA, NASA, and CNRS, France.

  9. High temperature pyrolysis to extract 36Cl for Accelerator Mass Spectrometry measurements

    NASA Astrophysics Data System (ADS)

    Cornett, R. J.; Andrews, H. R.; Chant, L.; Chaput, T.; Imahori, Y.; Jirovec, J.; Kramer, S.; Koslowsky, V. T.; Milton, G. M.; Milton, J. C. D.

    1996-10-01

    36Cl and stable Cl were extracted from solids by high temperature pyrolysis and then analyzed by Accelerator Mass Spectrometry (AMS). Cl was quantitatively extracted from rock, ore, vegetation and freshwater sediments in samples weighing from 100 mg to 2 g. 36Cl:Cl activity ratios measured following Cl extraction by pyrolysis agreed with those measured following Cl extraction by acid leaching. The simple pyrolysis extraction has the additional advantages that stable Cl - can be measured on the same sample along with other anions, the 36Cl:Cl ratio can be adjusted by diluting the known Cl - concentration in the collection solution to control the activity of 36Cl in the target and the potential interference of 36S can also be assessed prior to the AMS measurements.

  10. Precision neutron flux measurements and applications using the Alpha Gamma device

    NASA Astrophysics Data System (ADS)

    Anderson, Eamon; Alpha Gamma; BL2 Collaboration

    2015-04-01

    The Alpha Gamma device is a totally-absorbing 10 B neutron detector designed to measure the absolute detection efficiency of a thin-film lithium neutron monitor on a monoenergetic neutron beam. The detector has been shown to measure neutron fluence with an absolute accuracy of 0.06%. This capability has been used to perform the first direct, absolute measurement of the 6Li(n , t) 4He cross section at sub-thermal energy, improve the neutron fluence determination in a past beam neutron lifetime measurement by a factor of five, and is being used to calibrate the neutron monitors for use in the upcoming beam neutron lifetime measurement BL2 (NIST Beam Lifetime 2). The principle of the measurement method will presented and the applications will be discussed. We would like to acknowledge support of this research through the NSF-PHY-1068712 grant as well as the NIST Precision Measurement Grant program.

  11. Precision neutron flux measurements and applications using the Alpha Gamma device

    NASA Astrophysics Data System (ADS)

    Anderson, Eamon

    2016-03-01

    The Alpha Gamma device is a totally-absorbing 10 B neutron detector designed to measure the absolute detection efficiency of a thin-film lithium neutron monitor on a monoenergetic neutron beam. The detector has been shown to measure neutron fluence with an absolute accuracy of 0.06%. This capability has been used to perform the first direct, absolute measurement of the 6Li(n,t) 4He cross section at sub-thermal energy, improve the neutron fluence determination in a past beam neutron lifetime measurement by a factor of five, and is being used to calibrate the neutron monitors for use in the upcoming beam neutron lifetime measurement BL2 (NIST Beam Lifetime 2). The principle of the measurement method will presented and the applications will be discussed. We would like to acknowledge support of this research through the NSF-PHY-1068712 Grant as well as the NIST Precision Measurement Grant program.

  12. Gamma ray and fair weather electric field measurements during thunderstorms: indications for TGEs?

    NASA Astrophysics Data System (ADS)

    Reuveni, Yuval; Yair, Yoav; Steinitz, Gideon; Price, Colin; Pustil'nik, Lev; Yaniv, Roy; Hamiel, Yariv; Katz, Evgeni

    2016-04-01

    We report coincidences of ground-level gamma-ray enhancements with strong electric fields typical of lightning discharges, measured at a mountainous site in northern Israel. High-energy emissions detected on the Earth's surface during thunderstorms supposedly initiate Thunderstorm Ground Enhancements (TGEs) of fluxes of electrons, neutrons and gamma rays that can last tens of minutes. Such enhancements are thought to be related to Extensive Cloud Showers (ECSs) initiated between the main negative charge center and the lower positive charge pocket in mature thunderstorms (Chilingarian et al., 2015). The Cosmic Ray and Space Weather Center located at Mt. Hermon hosts a gamma ray detector alongside a continuous multi-parametric array consisting of a Global Navigation Satellite Systems (GNSS) geodetic receiver (for measuring Precipitable Water Vapor (PWV) and ionospheric Total Electron Content (TEC)), vertical atmospheric electric field (Ez) and current (Jz) and a neutron super monitor (for cosmic ray measurements). The diurnal variations in fair-weather conditions exhibit a clear 24-hour periodicity, related to the diurnal variation of atmospheric parameters. During several severe thunderstorms that occurred over Israel and near the Mt. Hermon station in October and November 2015, we recorded several instantaneous enhancements in the counts of Gamma rays, which lasted ten of minutes, and that coincided with peaks in the vertical electric field and current. Lightning data obtained from the Israeli Lightning Detection Network (ILDN) show that these peaks match the occurrences of close-by CG lightning discharges. This talk will present correlations between the properties of parent flashes and the observed peaks, and discuss possible mechanisms.

  13. An efficient method of measuring the 4 mm helmet output factor for the Gamma Knife

    NASA Astrophysics Data System (ADS)

    Ma, Lijun; Li, X. Allen; Yu, Cedric X.

    2000-03-01

    It is essential to have accurate measurements of the 4 mm helmet output factor in the treatment of trigeminal neuralgia patients using the Gamma Knife. Because of the small collimator size and the sharp dose gradient at the beam focus, this measurement is generally tedious and difficult. We have developed an efficient method of measuring the 4 mm helmet output factor using regular radiographic films. The helmet output factor was measured by exposing a single Kodak XV film in the standard Leksell spherical phantom using the 18 mm helmet with 30-40 of its plug collimators replaced by the 4 mm plug collimators. The 4 mm helmet output factor was measured to be 0.876 ± 0.009. This is in excellent agreement with our EGS4 Monte Carlo simulated value of 0.876 ± 0.005. This helmet output factor value also agrees with more tedious TLD, diode and radiochromic film measurements that were each obtained using two separate measurements with the 18 mm helmet and the 4 mm helmet respectively. The 4 mm helmet output factor measured by the diode was 0.884 ± 0.016, and the TLD measurement was 0.890 ± 0.020. The radiochromic film measured value was 0.870 ± 0.018. Because a single-exposure measurement was performed instead of a double-exposure measurement, most of the systematic errors that appeared in the double-exposure measurements due to experimental setup variations were cancelled out. Consequently, the 4 mm helmet output factor is more precisely determined by the single-exposure approach. Therefore, routine measurement and quality assurance of the 4 mm helmet output factor of the Gamma Knife could be efficiently carried out using the proposed single-exposure technique.

  14. A Canadian high-energy neutron spectrometry system for measurements in space.

    PubMed

    Jonkmans, G; Andrews, H R; Clifford, E T H; Frketich, G; Ing, H; Koslowsky, V T; Noulty, R A; Miller, R C; Zhou, Y; Mortimer, A; Peterson, D; Wilkinson, R

    2005-01-01

    Bubble Technology Industries Inc. (BTI), with the support of the Canadian Space Agency, has finished the construction of the Canadian High-Energy Neutron Spectrometry System (CHENSS). This spectrometer is intended to measure the high energy neutron spectrum (approximately 1-100 MeV) encountered in spacecraft in low earth orbit. CHENSS is designed to fly aboard a US space shuttle and its scientific results should facilitate the prediction of neutron dose to astronauts in space from readings of different types of radiation dosimeters that are being used in various missions.

  15. A Canadian high-energy neutron spectrometry system for measurements in space.

    PubMed

    Jonkmans, G; Andrews, H R; Clifford, E T H; Frketich, G; Ing, H; Koslowsky, V T; Noulty, R A; Miller, R C; Zhou, Y; Mortimer, A; Peterson, D; Wilkinson, R

    2005-01-01

    Bubble Technology Industries Inc. (BTI), with the support of the Canadian Space Agency, has finished the construction of the Canadian High-Energy Neutron Spectrometry System (CHENSS). This spectrometer is intended to measure the high energy neutron spectrum (approximately 1-100 MeV) encountered in spacecraft in low earth orbit. CHENSS is designed to fly aboard a US space shuttle and its scientific results should facilitate the prediction of neutron dose to astronauts in space from readings of different types of radiation dosimeters that are being used in various missions. PMID:15835056

  16. Measurements of sulfur compounds in CO 2 by diode laser atomic absorption spectrometry

    NASA Astrophysics Data System (ADS)

    Franzke, J.; Stancu, D. G.; Niemax, K.

    2003-07-01

    Two simple methods for the analysis of the total concentration of sulfur in CO 2 by diode laser atomic absorption spectrometry of excited, metastable sulfur atoms in a direct current discharge are presented. In the first method, the CO 2 sample gas is mixed with the plasma gas (Ar or He) while the second is based on reproducible measurements of the sulfur released from the walls in a helium discharge after being deposited as a result of operating the discharge in pure CO 2 sample gas. The detection limits obtained satisfy the requirements for the control of sulfur compounds in CO 2 used in the food and beverage industry.

  17. Electron attachment rate constant measurement by photoemission electron attachment ion mobility spectrometry (PE-EA-IMS)

    NASA Astrophysics Data System (ADS)

    Su, Desheng; Niu, Wenqi; Liu, Sheng; Shen, Chengyin; Huang, Chaoqun; Wang, Hongmei; Jiang, Haihe; Chu, Yannan

    2012-12-01

    Photoemission electron attachment ion mobility spectrometry (PE-EA-IMS), with a source of photoelectrons induced by vacuum ultraviolet radiation on a metal surface, has been developed to study electron attachment reaction at atmospheric pressure using nitrogen as the buffer gas. Based on the negative ion mobility spectra, the rate constants for electron attachment to tetrachloromethane and chloroform were measured at ambient temperature as a function of the average electron energy in the range from 0.29 to 0.96 eV. The experimental results are in good agreement with the data reported in the literature.

  18. Measurement uncertainty of isotopologue fractions in fluxomics determined via mass spectrometry.

    PubMed

    Guerrasio, R; Haberhauer-Troyer, C; Steiger, M; Sauer, M; Mattanovich, D; Koellensperger, G; Hann, S

    2013-06-01

    Metabolic flux analysis implies mass isotopomer distribution analysis and determination of mass isotopologue fractions (IFs) of proteinogenic amino acids of cell cultures. In this work, for the first time, this type of analysis is comprehensively investigated in terms of measurement uncertainty by calculating and comparing budgets for different mass spectrometric techniques. The calculations addressed amino acids of Pichia pastoris grown on 10% uniformly (13)C labeled glucose. Typically, such experiments revealed an enrichment of (13)C by at least one order of magnitude in all proteinogenic amino acids. Liquid chromatography-time-of-flight mass spectrometry (LC-TOFMS), liquid chromatography-tandem mass spectrometry (LC-MS/MS) and gas chromatography-mass spectrometry (GC-MS) analyses were performed. The samples were diluted to fit the linear dynamic range of the mass spectrometers used (10 μM amino acid concentration). The total combined uncertainties of IFs as well as the major uncertainty contributions affecting the IFs were determined for phenylalanine, which was selected as exemplary model compound. A bottom-up uncertainty propagation was performed according to Quantifying Uncertainty in Analytical Measurement and using the Monte Carlo method by considering all factors leading to an IF, i.e., the process of measurement and the addition of (13)C-glucose. Excellent relative expanded uncertainties (k = 1) of 0.32, 0.75, and 0.96% were obtained for an IF value of 0.7 by LC-MS/MS, GC-MS, and LC-TOFMS, respectively. The major source of uncertainty, with a relative contribution of 20-80% of the total uncertainty, was attributed to the signal intensity (absolute counts) uncertainty calculated according to Poisson counting statistics, regardless which of the mass spectrometry platforms was used. Uncertainty due to measurement repeatability was of importance in LC-MS/MS, showing a relative contribution up to 47% of the total uncertainty, whereas for GC-MS and LC

  19. Measurement of the K{sup +{yields}{pi}0{mu}+{nu}}{sub {mu}{gamma}}branching ratio

    SciTech Connect

    Adler, S.; Chiang, I-H.; Diwan, M. V.; Frank, J. S.; Haggerty, J. S.; Jaffe, D. E.; Jain, V.; Kettell, S. H.; Li, K. K.; Littenberg, L. S.; Ng, C.; Strand, R. C.; Witzig, C.; Bazarko, A. O.; Ito, M. M.; Meyers, P. D.; Shoemaker, F. C.; Stone, J. R.; Bergbusch, P. C.; Bryman, D. A.

    2010-05-01

    A measurement of the decay K{sup +{yields}{pi}0{mu}+{nu}}{sub {mu}{gamma}}has been performed with the E787 detector at Brookhaven National Laboratory. Forty events were observed in the signal region with the background expectation of (16.5{+-}2.7) events. The branching ratio was measured to be (1.58{+-}0.46(stat.){+-}0.08(syst.))x10{sup -5} in the kinematic region E{sub {gamma}>}30 MeV and {theta}{sub {mu}{gamma}>}20 deg., where E{sub {gamma}}is the energy of the emitted photon and {theta}{sub {mu}{gamma}}is the angle between the muon and the photon in the K{sup +} rest frame. The results were consistent with theoretical predictions.

  20. Semiquinone and ascorbyl radicals in the gut fluids of caterpillars measured with EPR spectrometry.

    PubMed

    Barbehenn, R V; Poopat, U; Spencer, B

    2003-01-01

    The biological activity of phenolic compounds ingested by caterpillars is commonly believed to result from their oxidation, although the products of oxidation have been well-characterized in only a few cases. The initial oxidation products of phenols (semiquinone or phenoxyl radicals) can be measured with electron paramagnetic resonance (EPR) spectrometry. In this study semiquinone radicals formed from tannic acid and gallic acid in the gut fluids of two species of caterpillars were measured. In Orgyia leucostigma, in which ingested phenols are not oxidized, semiquinone radicals were absent or at very low intensities. By contrast, in Malacosoma disstria, in which ingested phenols are oxidized, high semiquinone radical intensities were measured. In the absence of detectable levels of semiquinone radicals, ascorbyl radicals were detected in the EPR spectra instead. High molar ratios of ascorbate to phenols in an artificial diet produced ascorbyl radicals in the midgut fluids of both species, while diets containing low molar ratios produced semiquinone radicals. Similar results were obtained in M. disstria fed the leaves of red oak or sugar maple. The results of this study provide further evidence that ascorbate is an essential antioxidant that prevents the oxidation of phenols in the gut fluids of caterpillars, and demonstrate that EPR spectrometry is a valuable method for determining the degree of oxidative activation of phenols ingested by herbivorous insects. PMID:12459207

  1. ``Super'' Gas Cherenkov Detector for Gamma Ray Measurements at the National Ignition Facility

    NASA Astrophysics Data System (ADS)

    Herrmann, Hans W.; Kim, Y. H.; McEvoy, A. M.; Zylstra, A. B.; Lopez, F. E.; Griego, J. R.; Fatherley, V. E.; Oertel, J. A.; Batha, S. H.; Stoeffl, W.; Church, J. A.; Carpenter, A.; Rubery, M. S.; Horsfield, C. J.; Gales, S.; Leatherland, A.; Hilsabeck, T.; Kilkenny, J. D.; Malone, R. M.; Shmayda, W. T.

    2015-11-01

    New requirements to improve reaction history and ablator areal density measurements at the NIF necessitate improvements in sensitivity, temporal and spectral response relative to the existing Gamma Reaction History diagnostic (GRH-6m) located 6 meters from target chamber center (TCC). A new DIM-based ``Super'' Gas Cherenkov Detector (GCD) will ultimately provide ~ 200x more sensitivity to DT fusion gamma rays, reduce the effective temporal resolution from ~ 100 to ~ 10 ps and lower the energy threshold from 2.9 to 1.8 MeV, relative to GRH-6m. The first phase is to insert the existing coaxial GCD-3 detector into a reentrant well on the NIF chamber which will put it within 4 meters of TCC. This diagnostic platform will allow assessment of the x-ray radiation background environment within the well which will be fed into the shielding design for the follow-on ``Super'' GCD. It will also enable use of a pulse-dilation PMT which has the potential to improve the effective measurement bandwidth by ~ 10x relative to current PMT technology. GCD-3 has been thoroughly tested at the OMEGA Laser Facility and characterized at the High Intensity Gamma Ray Source (HIgS).

  2. Gamma rays and cosmic rays at Venus: The Pioneer Venus gamma ray detector and considerations for future measurements

    NASA Astrophysics Data System (ADS)

    Lorenz, Ralph D.; Lawrence, David J.

    2015-05-01

    We draw attention to, and present a summary archive of the data from, the Pioneer Venus Orbiter Gamma-ray Burst Detector (OGBD), an instrument not originally conceived with Venus science in mind. We consider the possibility of gamma-ray flashes generated by lightning and model the propagation of gamma rays in the Venusian atmosphere, finding that if gamma rays originate at the upper range of reported cloud top altitudes (75 km altitude), they may be attenuated by factors of only a few, whereas from 60 km altitude they are attenuated by over two orders of magnitude. The present archive is too heavily averaged to reliably detect such a source (and we appeal to investigators who may have retained a higher-resolution archive), but the data do provide a useful and unique record of the cosmic ray flux at Venus 1978-1993. We consider other applications of future orbital gamma ray data, such as atmospheric occultations and the detection of volcanic materials injected high in the atmosphere.

  3. Stellar and primordial nucleosynthesis of 7Be: measurement of 3He(alpha,gamma)7Be.

    PubMed

    Di Leva, A; Gialanella, L; Kunz, R; Rogalla, D; Schürmann, D; Strieder, F; De Cesare, M; De Cesare, N; D'Onofrio, A; Fülöp, Z; Gyürky, G; Imbriani, G; Mangano, G; Ordine, A; Roca, V; Rolfs, C; Romano, M; Somorjai, E; Terrasi, F

    2009-06-12

    The 3He(alpha,gamma)7Be reaction presently represents the largest nuclear uncertainty in the predicted solar neutrino flux and has important implications on the big bang nucleosynthesis, i.e., the production of primordial 7Li. We present here the results of an experiment using the recoil separator ERNA (European Recoil separator for Nuclear Astrophysics) to detect directly the 7Be ejectiles. In addition, off-beam activation and coincidence gamma-ray measurements were performed at selected energies. At energies above 1 MeV a large discrepancy compared to previous results is observed both in the absolute value and in the energy dependence of the cross section. Based on the available data and models, a robust estimate of the cross section at the astrophysical relevant energies is proposed. PMID:19658929

  4. Measurement of the branching fraction of Gamma(4S) --> B0B0.

    PubMed

    Aubert, B; Barate, R; Boutigny, D; Couderc, F; Karyotakis, Y; Lees, J P; Poireau, V; Tisserand, V; Zghiche, A; Grauges-Pous, E; Palano, A; Pappagallo, M; Pompili, A; Chen, J C; Qi, N D; Rong, G; Wang, P; Zhu, Y S; Eigen, G; Ofte, I; Stugu, B; Abrams, G S; Borgland, A W; Breon, A B; Brown, D N; Button-Shafer, J; Cahn, R N; Charles, E; Day, C T; Gill, M S; Gritsan, A V; Groysman, Y; Jacobsen, R G; Kadel, R W; Kadyk, J; Kerth, L T; Kolomensky, Yu G; Kukartsev, G; Lynch, G; Mir, L M; Oddone, P J; Orimoto, T J; Pripstein, M; Roe, N A; Ronan, M T; Wenzel, W A; Barrett, M; Ford, K E; Harrison, T J; Hart, A J; Hawkes, C M; Morgan, S E; Watson, A T; Fritsch, M; Goetzen, K; Held, T; Koch, H; Lewandowski, B; Pelizaeus, M; Peters, K; Schroeder, T; Steinke, M; Boyd, J T; Burke, J P; Chevalier, N; Cottingham, W N; Kelly, M P; Cuhadar-Donszelmann, T; Hearty, C; Knecht, N S; Mattison, T S; McKenna, J A; Thiessen, D; Khan, A; Kyberd, P; Teodorescu, L; Blinov, A E; Blinov, V E; Bukin, A D; Druzhinin, V P; Golubev, V B; Ivanchenko, V N; Kravchenko, E A; Onuchin, A P; Serednyakov, S I; Skovpen, Yu I; Solodov, E P; Yushkov, A N; Best, D; Bondioli, M; Bruinsma, M; Chao, M; Eschrich, I; Kirkby, D; Lankford, A J; Mandelkern, M; Mommsen, R K; Roethel, W; Stoker, D P; Buchanan, C; Hartfiel, B L; Weinstein, A J R; Foulkes, S D; Gary, J W; Long, O; Shen, B C; Wang, K; Zhang, L; Del Re, D; Hadavand, H K; Hill, E J; MacFarlane, D B; Paar, H P; Rahatlou, Sh; Sharma, V; Berryhill, J W; Campagnari, C; Cunha, A; Dahmes, B; Hong, T M; Lu, A; Mazur, M A; Richman, J D; Verkerke, W; Beck, T W; Eisner, A M; Flacco, C J; Heusch, C A; Kroseberg, J; Lockman, W S; Nesom, G; Schalk, T; Schumm, B A; Seiden, A; Spradlin, P; Williams, D C; Wilson, M G; Albert, J; Chen, E; Dubois-Felsmann, G P; Dvoretskii, A; Hitlin, D G; Narsky, I; Piatenko, T; Porter, F C; Ryd, A; Samuel, A; Yang, S; Jayatilleke, S; Mancinelli, G; Meadows, B T; Sokoloff, M D; Blanc, F; Bloom, P; Chen, S; Ford, W T; Nauenberg, U; Olivas, A; Rankin, P; Ruddick, W O; Smith, J G; Ulmer, K A; Zhang, J; Chen, A; Eckhart, E A; Harton, J L; Soffer, A; Toki, W H; Wilson, R J; Zeng, Q; Spaan, B; Altenburg, D; Brandt, T; Brose, J; Dickopp, M; Feltresi, E; Hauke, A; Lacker, H M; Maly, E; Nogowski, R; Otto, S; Petzold, A; Schott, G; Schubert, J; Schubert, K R; Schwierz, R; Sundermann, J E; Bernard, D; Bonneaud, G R; Grenier, P; Schrenk, S; Thiebaux, Ch; Vasileiadis, G; Verderi, M; Bard, D J; Clark, P J; Gradl, W; Muheim, F; Playfer, S; Xie, Y; Andreotti, M; Azzolini, V; Bettoni, D; Bozzi, C; Calabrese, R; Cibinetto, G; Luppi, E; Negrini, M; Piemontese, L; Sarti, A; Anulli, F; Baldini-Ferroli, R; Calcaterra, A; de Sangro, R; Finocchiaro, G; Patteri, P; Peruzzi, I M; Piccolo, M; Zallo, A; Buzzo, A; Capra, R; Contri, R; Lo Vetere, M; Macri, M; Monge, M R; Passaggio, S; Patrignani, C; Robutti, E; Santroni, A; Tosi, S; Bailey, S; Brandenburg, G; Chaisanguanthum, K S; Morii, M; Won, E; Dubitzky, R S; Langenegger, U; Marks, J; Uwer, U; Bhimji, W; Bowerman, D A; Dauncey, P D; Egede, U; Gaillard, J R; Morton, G W; Nash, J A; Nikolich, M B; Taylor, G P; Charles, M J; Grenier, G J; Mallik, U; Cochran, J; Crawley, H B; Meyer, W T; Prell, S; Rosenberg, E I; Rubin, A E; Yi, J; Arnaud, N; Davier, M; Giroux, X; Grosdidier, G; Höcker, A; Le Diberder, F; Lepeltier, V; Lutz, A M; Petersen, T C; Pierini, M; Plaszczynski, S; Rodier, S; Roudeau, P; Schune, M H; Stocchi, A; Wormser, G; Cheng, C H; Lange, D J; Simani, M C; Wright, D M; Bevan, A J; Chavez, C A; Coleman, J P; Forster, I J; Fry, J R; Gabathuler, E; Gamet, R; George, K A; Hutchcroft, D E; Parry, R J; Payne, D J; Touramanis, C; Cormack, C M; Di Lodovico, F; Brown, C L; Cowan, G; Flack, R L; Flaecher, H U; Green, M G; Jackson, P S; McMahon, T R; Ricciardi, S; Salvatore, F; Winter, M A; Brown, D; Davis, C L; Allison, J; Barlow, N R; Barlow, R J; Hodgkinson, M C; Lafferty, G D; Naisbit, M T; Williams, J C; Chen, C; Farbin, A; Hulsbergen, W D; Jawahery, A; Kovalskyi, D; Lae, C K; Lillard, V; Roberts, D A; Blaylock, G; Dallapiccola, C; Hertzbach, S S; Kofler, R; Koptchev, V B; Moore, T B; Saremi, S; Staengle, H; Willocq, S; Cowan, R; Koeneke, K; Sciolla, G; Sekula, S J; Taylor, F; Yamamoto, R K; Patel, P M; Robertson, S H; Lazzaro, A; Lombardo, V; Palombo, F; Bauer, J M; Cremaldi, L; Eschenburg, V; Godang, R; Kroeger, R; Reidy, J; Sanders, D A; Summers, D J; Zhao, H W; Brunet, S; Côté, D; Taras, P; Nicholson, H; Cavallo, N; De Nardo, G; Fabozzi, F; Gatto, C; Lista, L; Monorchio, D; Paolucci, P; Piccolo, D; Sciacca, C; Baak, M; Bulten, H; Raven, G; Snoek, H L; Wilden, L; Jessop, C P; Losecco, J M; Allmendinger, T; Benelli, G; Gan, K K; Honscheid, K; Hufnagel, D; Kagan, H; Kass, R; Pulliam, T; Rahimi, A M; Ter-Antonyan, R; Wong, Q K; Brau, J; Frey, R; Igonkina, O; Lu, M; Potter, C T; Sinev, N B; Strom, D; Torrence, E; Colecchia, F; Dorigo, A; Galeazzi, F; Margoni, M; Morandin, M; Posocco, M; Rotondo, M; Simonetto, F; Stroili, R; Voci, C; Benayoun, M; Briand, H; Chauveau, J; David, P; Del Buono, L; de la Vaissière, Ch; Hamon, O; John, M J J; Leruste, Ph; Malclès, J; Ocariz, J; Roos, L; Therin, G; Behera, P K; Gladney, L; Guo, Q H; Panetta, J; Biasini, M; Covarelli, R; Pioppi, M; Angelini, C; Batignani, G; Bettarini, S; Bucci, F; Calderini, G; Carpinelli, M; Forti, F; Giorgi, M A; Lusiani, A; Marchiori, G; Morganti, M; Neri, N; Paoloni, E; Rama, M; Rizzo, G; Simi, G; Walsh, J; Haire, M; Judd, D; Paick, K; Wagoner, D E; Danielson, N; Elmer, P; Lau, Y P; Lu, C; Olsen, J; Smith, A J S; Telnov, A V; Bellini, F; Cavoto, G; D'Orazio, A; Di Marco, E; Faccini, R; Ferrarotto, F; Ferroni, F; Gaspero, M; Li Gioi, L; Mazzoni, M A; Morganti, S; Piredda, G; Polci, F; Tehrani, F Safai; Voena, C; Christ, S; Schröder, H; Wagner, G; Waldi, R; Adye, T; De Groot, N; Franek, B; Gopal, G P; Olaiya, E O; Wilson, F F; Aleksan, R; Emery, S; Gaidot, A; Ganzhur, S F; Giraud, P-F; Graziani, G; de Monchenault, G Hamel; Kozanecki, W; Legendre, M; London, G W; Mayer, B; Vasseur, G; Yèche, Ch; Zito, M; Purohit, M V; Weidemann, A W; Wilson, J R; Yumiceva, F X; Abe, T; Allen, M; Aston, D; Bartoldus, R; Berger, N; Boyarski, A M; Buchmueller, O L; Claus, R; Convery, M R; Cristinziani, M; Dingfelder, J C; Dong, D; Dorfan, J; Dujmic, D; Dunwoodie, W; Fan, S; Field, R C; Glanzman, T; Gowdy, S J; Hadig, T; Halyo, V; Hast, C; Hryn'ova, T; Innes, W R; Kelsey, M H; Kim, P; Kocian, M L; Leith, D W G S; Libby, J; Luitz, S; Luth, V; Lynch, H L; Marsiske, H; Messner, R; Mohapatra, A K; Muller, D R; O'Grady, C P; Ozcan, V E; Perazzo, A; Perl, M; Ratcliff, B N; Roodman, A; Salnikov, A A; Schindler, R H; Schwiening, J; Snyder, A; Soha, A; Stelzer, J; Strube, J; Su, D; Sullivan, M K; Thompson, J; Va'vra, J; Wagner, S R; Weaver, M; Wisniewski, W J; Wittgen, M; Wright, D H; Yarritu, A K; Young, C C; Burchat, P R; Edwards, A J; Majewski, S A; Petersen, B A; Roat, C; Ahmed, M; Ahmed, S; Alam, M S; Ernst, J A; Saeed, M A; Saleem, M; Wappler, F R; Bugg, W; Krishnamurthy, M; Spanier, S M; Eckmann, R; Kim, H; Ritchie, J L; Satpathy, A; Schwitters, R F; Izen, J M; Kitayama, I; Lou, X C; Ye, S; Bianchi, F; Bona, M; Gallo, F; Gamba, D; Bomben, M; Bosisio, L; Cartaro, C; Cossutti, F; Ricca, G Della; Dittongo, S; Grancagnolo, S; Lanceri, L; Poropat, P; Vitale, L; Vuagnin, G; Martinez-Vidal, F; Panvini, R S; Banerjee, Sw; Bhuyan, B; Brown, C M; Fortin, D; Hamano, K; Jackson, P D; Kowalewski, R; Roney, J M; Sobie, R J; Back, J J; Harrison, P F; Latham, T E; Mohanty, G B; Band, H R; Chen, X; Cheng, B; Dasu, S; Datta, M; Eichenbaum, A M; Flood, K T; Graham, M; Hollar, J J; Johnson, J R; Kutter, P E; Li, H; Liu, R; Mellado, B; Mihalyi, A; Pan, Y; Prepost, R; Tan, P; von Wimmersperg-Toeller, J H; Wu, J; Wu, S L; Yu, Z; Greene, M G; Neal, H

    2005-07-22

    We report the first measurement of the branching fraction f(00) for Gamma(4S) --> B(0)B(0). The data sample consists of 81.7 fb(-1) collected at the Gamma(4S) resonance with the BABAR detector at the SLAC PEP-II asymmetric-energy e(+)e(-) storage ring. Using partial reconstruction of the decay B(0) --> D(*+) l(-)nu(l) in which only the charged lepton and the soft pion from the decay D(*+) --> D(0)pi(+) are reconstructed, we obtain f(00) = 0.487 +/- 0.010(stat) +/- 0.008(syst). Our result does not depend on the branching fractions of B(0) --> D(*+)l(-)nu(l) and D(*+) --> D(0)pi(+) decays, on the ratio of the charged and neutral B meson lifetimes, nor on the assumption of isospin symmetry.

  5. Stellar and primordial nucleosynthesis of 7Be: measurement of 3He(alpha,gamma)7Be.

    PubMed

    Di Leva, A; Gialanella, L; Kunz, R; Rogalla, D; Schürmann, D; Strieder, F; De Cesare, M; De Cesare, N; D'Onofrio, A; Fülöp, Z; Gyürky, G; Imbriani, G; Mangano, G; Ordine, A; Roca, V; Rolfs, C; Romano, M; Somorjai, E; Terrasi, F

    2009-06-12

    The 3He(alpha,gamma)7Be reaction presently represents the largest nuclear uncertainty in the predicted solar neutrino flux and has important implications on the big bang nucleosynthesis, i.e., the production of primordial 7Li. We present here the results of an experiment using the recoil separator ERNA (European Recoil separator for Nuclear Astrophysics) to detect directly the 7Be ejectiles. In addition, off-beam activation and coincidence gamma-ray measurements were performed at selected energies. At energies above 1 MeV a large discrepancy compared to previous results is observed both in the absolute value and in the energy dependence of the cross section. Based on the available data and models, a robust estimate of the cross section at the astrophysical relevant energies is proposed.

  6. Measurements with Pinhole and Coded Aperture Gamma-Ray Imaging Systems

    SciTech Connect

    Raffo-Caiado, Ana Claudia; Solodov, Alexander A; Abdul-Jabbar, Najeb M; Hayward, Jason P; Ziock, Klaus-Peter

    2010-01-01

    From a safeguards perspective, gamma-ray imaging has the potential to reduce manpower and cost for effectively locating and monitoring special nuclear material. The purpose of this project was to investigate the performance of pinhole and coded aperture gamma-ray imaging systems at Oak Ridge National Laboratory (ORNL). With the aid of the European Commission Joint Research Centre (JRC), radiometric data will be combined with scans from a three-dimensional design information verification (3D-DIV) system. Measurements were performed at the ORNL Safeguards Laboratory using sources that model holdup in radiological facilities. They showed that for situations with moderate amounts of solid or dense U sources, the coded aperture was able to predict source location and geometry within ~7% of actual values while the pinhole gave a broad representation of source distributions

  7. Radial Electron Temperature and Density Measurements Using Thomson Scattering System in GAMMA 10/PDX

    NASA Astrophysics Data System (ADS)

    Yoshikawa, M.; Ohta, K.; Wang, X.; Chikatsu, M.; Kohagura, J.; Shima, Y.; Sakamoto, M.; Imai, T.; Nakashima, Y.; Yasuhara, R.; Yamada, I.; Funaba, H.; Minami, T.

    2015-11-01

    A Thomson scattering (TS) system in GAMMA 10/PDX has been developed for the measurement of radial profiles of electron temperature and density in a single plasma and laser shot. The TS system has a large solid angle optical collection system and high-sensitivity signal detection system. The TS signals are obtained using four-channel high-speed digital oscilloscopes controlled by a Windows PC. We designed the acquisition program for six oscilloscopes to obtain 10-Hz TS signals in a single plasma shot, following which the time-dependent electron temperatures and densities can be determined. Moreover, in order to obtain larger TS signal intensity in the edge region, we added a second collection mirror. The radial electron temperatures and densities at six radial positions in GAMMA 10/PDX were successfully obtained.

  8. Time-resolved spectroscopy measurements of hydrogen-alpha, -beta, and -gamma emissions

    SciTech Connect

    Parigger, Christian G.; Dackman, Matthew; Hornkohl, James O

    2008-11-01

    Hydrogen emission spectroscopy results are reported following laser-induced optical breakdown with infrared Nd:YAG laser radiation focused into a pulsed methane flow. Measurements of Stark-broadened atomic hydrogen-alpha, -beta, and -gamma lines show electron number densities of 0.3 to 4x10{sup 17} cm{sup -3} for time delays of 2.1 to 0.4 {mu}s after laser-induced optical breakdown. In methane flow, recombination molecular spectra of the {delta}{nu}=+2 progression of the C2 Swan system are discernable in the H{beta} and H{gamma} plasma emissions within the first few microseconds. The recorded atomic spectra indicate the occurrence of hydrogen self-absorption for pulsed CH4 flow pressures of 2.7x10{sup 5} Pa (25 psig) and 6.5x10{sup 5} Pa (80 psig)

  9. Standardization and measurement of gamma-ray probability per decay of 177Lu.

    PubMed

    Dias, Mauro S; Silva, Fabrício F V; Koskinas, Marina F

    2010-01-01

    The procedure followed by the Nuclear Metrology Laboratory (LMN), at the Nuclear and Energy Research Institute (IPEN), for the primary standardization of (177)Lu is described. This radionuclide is widely used in radiopharmacy due to its convenient half-life and emitted beta ray energies. The (177)Lu solution was supplied during an international comparison sponsored by BIPM in 2009 and the primary standardization has been accomplished by the 4pibeta-gamma coincidence method using a proportional counter in 4pi geometry coupled with two NaI(Tl) scintillation counters. The beta efficiency was varied by placing Collodion and aluminum absorbers over and under the radioactive source. The (177)Lu calibrated sources were also measured in a previously calibrated HPGe spectrometer, in order to obtain the emission probability per decay for the selected gamma-ray transitions. The experimental extrapolation curves were also compared with Monte Carlo simulations by means of code ESQUEMA developed at the LMN.

  10. Measurements of neutron distribution in neutrons-gamma-rays mixed field using imaging plate for neutron capture therapy.

    PubMed

    Tanaka, Kenichi; Endo, Satoru; Hoshi, Masaharu

    2010-01-01

    The imaging plate (IP) technique is tried to be used as a handy method to measure the spatial neutron distribution via the (157)Gd(n,gamma)(158)Gd reaction for neutron capture therapy (NCT). For this purpose, IP is set in a water phantom and irradiated in a mixed field of neutrons and gamma-rays. The Hiroshima University Radiobiological Research Accelerator is utilized for this experiment. The neutrons are moderated with 20-cm-thick D(2)O to obtain suitable neutron field for NCT. The signal for IP doped with Gd as a neutron-response enhancer is subtracted with its contribution by gamma-rays, which was estimated using IP without Gd. The gamma-ray response of Gd-doped IP to non-Gd IP is set at 1.34, the value measured for (60)Co gamma-rays, in estimating the gamma-ray contribution to Gd-doped IP signal. Then measured distribution of the (157)Gd(n,gamma)(158)Gd reaction rate agrees within 10% with the calculated value based on the method that has already been validated for its reproducibility of Au activation. However, the evaluated distribution of the (157)Gd(n,gamma)(158)Gd reaction rate is so sensitive to gamma-ray energy, e.g. the discrepancy of the (157)Gd(n,gamma)(158)Gd reaction rate between measurement and calculation becomes 30% for the photon energy change from 33keV to 1.253MeV.

  11. Measurement of Parity-Violating Neutron Capture Gamma Asymmetries at Low-Energies

    SciTech Connect

    Barron-Palos, L.; Bowman, James D; Fomin, Nadia; Greene, G. L.; Penttila, Seppo I

    2009-01-01

    A sensitive measurement of parity-violating (PV) observables in few-nucleon systems can shed light on our current understanding of the hadronic weak interaction at low momentum transfers. Theoretical models describe the nucleon-nucleon weak interaction at low energies with 6 parameters that need, in principle, to be determined in the same number of independent experiments. In this context, a series of experiments with cold neutrons are being proposed and developed. Particularly, experiments that aim to measure the parity-violating asymmetry in the distribution of the gamma-rays emitted in the capture of polarized neutrons by protons and deuterium, will be discussed in this paper.

  12. Measurement of total-body cobalt-57 vitamin B12 absorption with a gamma camera.

    PubMed

    Cardarelli, J A; Slingerland, D W; Burrows, B A; Miller, A

    1985-08-01

    Previously described techniques for the measurement of the absorption of [57Co]vitamin B12 by total-body counting have required an iron room equipped with scanning or multiple detectors. The present study uses simplifying modifications which make the technique more available and include the use of static geometry, the measurement of body thickness to correct for attenuation, a simple formula to convert the capsule-in-air count to a 100% absorption count, and finally the use of an adequately shielded gamma camera obviating the need of an iron room.

  13. Simulation and Measurement of Absorbed Dose from 137 Cs Gammas Using a Si Timepix Detector

    NASA Technical Reports Server (NTRS)

    Stoffle, Nicholas; Pinsky, Lawrence; Empl, Anton; Semones, Edward

    2011-01-01

    The TimePix readout chip is a hybrid pixel detector with over 65k independent pixel elements. Each pixel contains its own circuitry for charge collection, counting logic, and readout. When coupled with a Silicon detector layer, the Timepix chip is capable of measuring the charge, and thus energy, deposited in the Silicon. Measurements using a NIST traceable 137Cs gamma source have been made at Johnson Space Center using such a Si Timepix detector, and this data is compared to simulations of energy deposition in the Si layer carried out using FLUKA.

  14. Measurements of the angles {alpha} and {gamma} of the CKM unitarity triangle with the BABAR experiment

    SciTech Connect

    Malcles, Julie

    2006-07-11

    Measurements of the modes B {yields} {pi}{pi} and B {yields} {rho}{rho} and their implications on the angle a of the CKM unitarity triangle are presented. Results of the Dalitz analysis of the modes B {yields} D(*)0K(*) and the derived constraints on the angle {gamma} are then shown. These measurements are based on a sample of approximately 230.106 B pairs taken at the {upsilon}(4S) resonance collected by the BABAR detector at the PEP-II asymmetric-energy beam factory at SLAC.

  15. Estimates of rates and errors for measurements of direct-{gamma} and direct-{gamma} + jet production by polarized protons at RHIC

    SciTech Connect

    Beddo, M.E.; Spinka, H.; Underwood, D.G.

    1992-08-14

    Studies of inclusive direct-{gamma} production by pp interactions at RHIC energies were performed. Rates and the associated uncertainties on spin-spin observables for this process were computed for the planned PHENIX and STAR detectors at energies between {radical}s = 50 and 500 GeV. Also, rates were computed for direct-{gamma} + jet production for the STAR detector. The goal was to study the gluon spin distribution functions with such measurements. Recommendations concerning the electromagnetic calorimeter design and the need for an endcap calorimeter for STAR are made.

  16. The LLNL Accelerator Mass Spectrometry System for Biochemical 14C-Measurements

    SciTech Connect

    Ognibene, T J; Bench, G; Brown, T A; Vogel, J S

    2002-10-31

    We report on recent improvements made to our 1 MV accelerator mass spectrometry system that is dedicated to {sup 14}C quantification of biochemical samples. Increased vacuum pumping capacity near the high voltage terminal has resulted in a 2-fold reduction of system backgrounds to 0.04 amol {sup 14}C/mg carbon. Carbon ion transmission through the accelerator has also improved a few percent. We have also developed tritium measurement capability on this spectrometer. The {sup 3}H/{sup 1}H isotopic ratio of a milligram-sized processed tap water sample has been measured at 4 {+-} 1 x 10{sup -16} (430 {+-} 110 {micro}Bq/mg H). Measurement throughput for a typical biochemical {sup 3}H sample is estimated to be {approx}10 minutes/sample.

  17. [Combustion temperature measurement of pyrotechnic composition using remote sensing Fourier transform infrared spectrometry].

    PubMed

    Zhou, Xin-li; Li, Yan; Liu, Zu-liang; Zhu, Chang-jiang; Wang, Jun-de; Lu, Chun-xu

    2002-10-01

    In this paper, combustion characterization of pyrotechnic composition is investigated using a remote sensing Fourier transform infrared spectrometry. The emission spectra have been recorded between 4,700 and 740 cm-1 with a spectral resolution of 4 cm-1. The combustion temperature can be determined remotely from spectral line intensity distribution of the fine structure of the emission fundamental band of gaseous products such as HF. The relationship between combustion temperature and combustion time has been given. Results show that there is a violent mutative temperature field with bigger temperature gradient near combustion surface. It reveals that the method of temperature measurement using remote sensing FTIR for flame temperature of unstable, violent and short time combustion on real time is a rapid, accurate and sensitive technique without interference the flame temperature field. Potential prospects of temperature measurement, gas product concentration measurement and combustion mechanism are also revealed.

  18. Gamma-ray thermoluminescence measurements: a record of fallout deposition in Hiroshima?

    PubMed

    Egbert, Stephen D; Kerr, George D

    2012-05-01

    In certain Hiroshima neighborhoods, radiation measurements using thermoluminescence dosimetry (TLD) exceed what can be explained by the initial gamma-ray doses and uncertainties from the Dosimetry System 2002 (DS02). This problem was not previously recognized as being isolated to certain parts of that city. The ratio between TLD measurements and DS02 dose calculations for gamma rays appear to grow larger than unity up to more than three with increasing ground range, but closer examination shows the excess TLD dose (0.1, 0.2, or possibly up to 0.8 Gray) is correlated with certain neighborhoods and could be due to radioactive fallout. At Nagasaki, the TLD measurements do not show this same excess, probably because there were no TLD measurements taken more than 800 m downwind (eastward) from the Nagasaki hypocenter, so that any small excess TLD dose was masked by larger initial gamma-ray doses of 25-80 Gray in the few downwind samples. The DS02 Report had noted many measurements lower than the DS02 calculation for several Nagasaki TLD samples, independent of ground range. This was explained as being the result of previously unaccounted urban shielding which was observed from Nagasaki pre-bomb aerial photos. However, the Hiroshima excess TLD dose issue was not resolved. If the excess TLD doses at Hiroshima are an indication of fallout, it may be possible to use additional TLD studies to make better estimates of the locations and radiation doses to survivors from the fallout after the bombings at both cities.

  19. New insights into the global composition of the lunar surface from high-energy gamma rays measured by Lunar Prospector

    NASA Astrophysics Data System (ADS)

    Peplowski, Patrick N.; Lawrence, David J.

    2013-04-01

    An analysis of the lunar gamma-ray spectrum as measured by the Lunar Prospector Gamma-Ray Spectrometer has revealed that 8-8.9 MeV gamma rays contain information about the elemental composition of near-surface materials. These high-energy gamma rays are found to be primarily sensitive to the total Fe and Mg content of the surface, although other elements also contribute. This information has been used to identify several regions with unique compositions, including the Hertzsprung and Orientale basins. A method for deriving global Mg abundances from high-energy gamma-ray measurements is presented. The physical mechanism for high-energy gamma-ray production is proposed to be radiation produced during the decay of galactic cosmic ray produced pions within the lunar surface. Laboratory measurements of pion production cross sections are found to be consistent with the empirically derived relationship between the lunar Fe, Mg, and Ti abundances and the measured high-energy gamma-ray count rates.

  20. Ultra-High Rate Measurements of Spent Fuel Gamma-Ray Emissions

    NASA Astrophysics Data System (ADS)

    Rodriguez, Douglas; Vandevender, Brent; Wood, Lynn; Glasgow, Brian; Taubman, Matthew; Wright, Michael; Dion, Michael; Pitts, Karl; Runkle, Robert; Campbell, Luke; Fast, James

    2014-03-01

    Presently there are over 200,000 irradiated spent nuclear fuel (SNF) assemblies in the world, each containing a concerning amount of weapons-usable material. Both facility operators and safeguards inspectors want to improve composition determination. Current measurements are expensive and difficult so new methods are developed through models. Passive measurements are limited since a few specific decay products and the associated down-scatter overwhelm the gamma rays of interest. Active interrogation methods produce gamma rays beyond 3 MeV, minimizing the impact of the passive emissions that drop off sharply above this energy. New devices like the Ultra-High Rate Germanium (UHRGe) detector are being developed to advance these novel measurement methods. Designed for reasonable resolution at 106 s-1 output rates (compared to ~ 1 - 10 e 3 s-1 standards), SNF samples were directly measured using UHRGe and compared to models. Model verification further enables using Los Alamos National Laboratory SNF assembly models, developed under the Next Generation Safeguards Initiative, to determine emission and signal expectations. Measurement results and future application requirements for UHRGe will be discussed.

  1. Measured Activities of Al and Ni in gamma-(Ni) and gamma'-(Ni)3Al in the Ni-Al-Pt System

    NASA Technical Reports Server (NTRS)

    Copland, Evan

    2007-01-01

    Adding Pt to Ni-Al coatings is critical to achieving the required oxidation protection of Ni-based superalloys, but the nature of the Pt effect remains unresolved. This research provides a fundamental part of the answer by measuring the influence of Pt on the activities of Al and Ni in gamma-(Ni), gamma prime-(Ni)3Al and liquid in the Ni-Al-Pt system. Measurements have been made at 25 compositions in the Ni-rich corner over the temperature range, T = 1400-1750 K, by the vapor pressure technique with a multiple effusion-cell mass spectrometer (multi-cell KEMS). These measurements clearly show adding Pt (for X(sub Pt) less than 0.25) decreases a(Al) while increasing a(Ni). This solution behavior supports the idea that Pt increases Al transport to an alloy / Al2O3 interface and also limits the interaction between the coating and substrate alloys in the gamma-(Ni) + gamma prime-(Ni)3Al region. This presentation will review the progress of this study.

  2. Intercomparison study on (152)Eu gamma ray and (36)Cl AMS measurements for development of the new Hiroshima-Nagasaki Atomic Bomb Dosimetry System 2002 (DS02).

    PubMed

    Hoshi, M; Endo, S; Tanaka, K; Ishikawa, M; Straume, T; Komura, K; Rühm, W; Nolte, E; Huber, T; Nagashima, Y; Seki, R; Sasa, K; Sueki, K; Fukushima, H; Egbert, S D; Imanaka, T

    2008-07-01

    In the process of developing a new dosimetry system for atomic bomb survivors in Hiroshima and Nagasaki (DS02), an intercomparison study between (152)Eu and (36)Cl measurements was proposed, to reconcile the discrepancy previously observed in the Hiroshima data between measurements and calculations of thermal neutron activation products. Nine granite samples, exposed to the atomic-bomb radiation in Hiroshima within 1,200 m of the hypocenter, as well as mixed standard solutions containing known amounts of europium and chlorine that were neutron-activated by a (252)Cf source, were used for the intercomparison. Gamma-ray spectrometry for (152)Eu was carried out with ultra low-background Ge detectors at the Ogoya Underground Laboratory, Kanazawa University, while three laboratories participated in the (36)Cl measurement using accelerator mass spectrometry (AMS): The Technical University of Munich, Germany, the Lawrence Livermore National Laboratory, USA and the University of Tsukuba, Japan. Measured values for the mixed standard solutions showed good agreement among the participant laboratories. They also agreed well with activation calculations, using the neutron fluences monitored during the (252)Cf irradiation, and the corresponding activation cross-sections taken from the JENDL-3.3 library. The measured-to-calculated ratios obtained were 1.02 for (152)Eu and 0.91-1.02 for (36)Cl, respectively. Similarly, the results of the granite intercomparison indicated good agreement with the DS02 calculation for these samples. An average measured-to-calculated ratio of 0.98 was obtained for all granite intercomparison measurements. The so-called neutron discrepancy that was previously observed and that which included increasing measured-to-calculated ratios for thermal neutron activation products for increasing distances beyond 1,000 m from the hypocenter was not seen in the results of the intercomparison study. The previously claimed discrepancy could be explained by

  3. Investigation of (235)U, (226)Ra, (232)Th, (40)K, (137)Cs, and heavy metal concentrations in Anzali international wetland using high-resolution gamma-ray spectrometry and atomic absorption spectroscopy.

    PubMed

    Zare, Mohammad Reza; Kamali, Mahdi; Fallahi Kapourchali, Maryam; Bagheri, Hashem; Khoram Bagheri, Mahdi; Abedini, Ali; Pakzad, Hamid Reza

    2016-02-01

    Measurements of natural radioactivity levels and heavy metals in sediment and soil samples of the Anzali international wetland were carried out by two HPGe-gamma ray spectrometry and atomic absorption spectroscopy techniques. The concentrations of (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs in sediment samples ranged between 1.05 ± 0.51-5.81 ± 0.61, 18.06 ± 0.63-33.36 ± .0.34, 17.57 ± 0.38-45.84 ± 6.23, 371.88 ± 6.36-652.28 ± 11.60, and 0.43 ± 0.06-63.35 ± 0.94 Bq/kg, while in the soil samples they vary between 2.36-5.97, 22.71-38.37, 29.27-42.89, 472.66-533, and 1.05-9.60 Bq/kg for (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs, respectively. Present results are compared with the available literature data and also with the world average values. The radium equivalent activity was well below the defined limit of 370 Bq/kg. The external hazard indices were found to be less than 1, indicating a low dose. Heavy metal concentrations were found to decrease in order as Fe > Mn > Sr > Zn > Cu > Cr > Ni > Pb > Co > Cd. These measurements will serve as background reference levels for the Anzali wetland. PMID:26490904

  4. Investigation of (235)U, (226)Ra, (232)Th, (40)K, (137)Cs, and heavy metal concentrations in Anzali international wetland using high-resolution gamma-ray spectrometry and atomic absorption spectroscopy.

    PubMed

    Zare, Mohammad Reza; Kamali, Mahdi; Fallahi Kapourchali, Maryam; Bagheri, Hashem; Khoram Bagheri, Mahdi; Abedini, Ali; Pakzad, Hamid Reza

    2016-02-01

    Measurements of natural radioactivity levels and heavy metals in sediment and soil samples of the Anzali international wetland were carried out by two HPGe-gamma ray spectrometry and atomic absorption spectroscopy techniques. The concentrations of (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs in sediment samples ranged between 1.05 ± 0.51-5.81 ± 0.61, 18.06 ± 0.63-33.36 ± .0.34, 17.57 ± 0.38-45.84 ± 6.23, 371.88 ± 6.36-652.28 ± 11.60, and 0.43 ± 0.06-63.35 ± 0.94 Bq/kg, while in the soil samples they vary between 2.36-5.97, 22.71-38.37, 29.27-42.89, 472.66-533, and 1.05-9.60 Bq/kg for (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs, respectively. Present results are compared with the available literature data and also with the world average values. The radium equivalent activity was well below the defined limit of 370 Bq/kg. The external hazard indices were found to be less than 1, indicating a low dose. Heavy metal concentrations were found to decrease in order as Fe > Mn > Sr > Zn > Cu > Cr > Ni > Pb > Co > Cd. These measurements will serve as background reference levels for the Anzali wetland.

  5. Measurements of gamma radiation levels and spectra in the San Francisco Bay Area

    NASA Astrophysics Data System (ADS)

    Lo, B. T.; Brozek, K. P.; Angell, C. T.; Norman, E. B.

    2011-10-01

    Much of the radiation received by an average person is emitted by naturally-occurring radioactive isotopes from the thorium, actinium, and uranium decay series, or potassium. In this study, we have measured gamma radiation levels at various locations in the San Francisco Bay Area and the UC Berkeley campus from spectra taken using an ORTEC NOMAD portable data acquisition system and a large-volume coaxial HPGe detector. We have identified a large number of gamma rays originating from natural sources. The most noticeable isotopes are 214Bi, 40K, and 208Tl. We have observed variations in counting rates by factors of two to five between different locations due to differences in local conditions - such as building, concrete, grass, and soil compositions. In addition, in a number of outdoor locations, we have observed 604-, 662-, and 795-keV gamma rays from 134,137Cs, which we attribute to fallout from the recent Fukushima reactor accident. The implications of these results will be discussed. This work was supported in part by a grant from the U. S. Dept. of Homeland Security.

  6. Statistical approaches to forecast gamma dose rates by using measurements from the atmosphere.

    PubMed

    Jeong, Hyo-Joon; Hwang, Won-Tae; Kim, Eun-Han; Han, Moon-Hee

    2008-01-01

    In this paper, the results obtained by inter-comparing several statistical techniques for estimating gamma dose rates, such as an exponential moving average model, a seasonal exponential smoothing model and an artificial neural networks model, are reported. Seven years of gamma dose rates data measured in Daejeon City, Korea, were divided into two parts to develop the models and validate the effectiveness of the generated predictions by the techniques mentioned above. Artificial neural networks model shows the best forecasting capability among the three statistical models. The reason why the artificial neural networks model provides a superior prediction to the other models would be its ability for a non-linear approximation. To replace the gamma dose rates when missing data for an environmental monitoring system occurs, the moving average model and the seasonal exponential smoothing model can be better because they are faster and easier for applicability than the artificial neural networks model. These kinds of statistical approaches will be helpful for a real-time control of radio emissions or for an environmental quality assessment.

  7. Component Activity Measurements in the Ti-Al-O System by Knudsen Cell Mass Spectrometry

    NASA Technical Reports Server (NTRS)

    Copland, Evan; Jacobson, Nathan S.

    2003-01-01

    Titanium-aluminides (containing (alpha)2-Ti3Al and gamma-TiAl intermetallic phases) have received continued research focus due to their potential as low-density materials for structural applications at intermediate temperatures. However their application above about 850C is hindered by poor oxidation resistance, characterized by the formation of a non-protective TiO2+Al2O3 scale and an oxygen-enriched subsurface zone. Consistent with this are measured titanium and aluminum activities in "oxygen-free" titanium-aluminides, which indicate Al2O3 is only stable for aluminum concentrations greater then 54 atom percent at 1373 K. However, the inability to form a protective Al2O3 scale is in apparent conflict with phase diagram studies, as experimental isothermal sections of the Ti-Al-O system show gamma-TiAl + alpha2-Ti3Al structures are in equilibrium only with Al2O3. The apparent resolution to this conflict lies in the inclusion of oxygen effects in the thermodynamic measurements

  8. Measurement of (233)U/(234)U ratios in contaminated groundwater using alpha spectrometry.

    PubMed

    Harrison, Jennifer J; Payne, Timothy E; Wilsher, Kerry L; Thiruvoth, Sangeeth; Child, David P; Johansen, Mathew P; Hotchkis, Michael A C

    2016-01-01

    The uranium isotope (233)U is not usually observed in alpha spectra from environmental samples due to its low natural and fallout abundance. It may be present in samples from sites in the vicinity of nuclear operations such as reactors or fuel reprocessing facilities, radioactive waste disposal sites or sites affected by clandestine nuclear operations. On an alpha spectrum, the two most abundant alpha emissions of (233)U (4.784 MeV, 13.2%; and 4.824 MeV, 84.3%) will overlap with the (234)U doublet peak (4.722 MeV, 28.4%; and 4.775 MeV, 71.4%), if present, resulting in a combined (233+234)U multiplet. A technique for quantifying both (233)U and (234)U from alpha spectra was investigated. A series of groundwater samples were measured both by accelerator mass spectrometry (AMS) to determine (233)U/(234)U atom and activity ratios and by alpha spectrometry in order to establish a reliable (233)U estimation technique using alpha spectra. The Genie™ 2000 Alpha Analysis and Interactive Peak Fitting (IPF) software packages were used and it was found that IPF with identification of three peaks ((234)U minor, combined (234)U major and (233)U minor, and (233)U major) followed by interference correction on the combined peak and a weighted average activity calculation gave satisfactory agreement with the AMS data across the (233)U/(234)U activity ratio range (0.1-20) and (233)U activity range (2-300 mBq) investigated. Correlation between the AMS (233)U and alpha spectrometry (233)U was r(2) = 0.996 (n = 10). PMID:26359847

  9. Measurement of (233)U/(234)U ratios in contaminated groundwater using alpha spectrometry.

    PubMed

    Harrison, Jennifer J; Payne, Timothy E; Wilsher, Kerry L; Thiruvoth, Sangeeth; Child, David P; Johansen, Mathew P; Hotchkis, Michael A C

    2016-01-01

    The uranium isotope (233)U is not usually observed in alpha spectra from environmental samples due to its low natural and fallout abundance. It may be present in samples from sites in the vicinity of nuclear operations such as reactors or fuel reprocessing facilities, radioactive waste disposal sites or sites affected by clandestine nuclear operations. On an alpha spectrum, the two most abundant alpha emissions of (233)U (4.784 MeV, 13.2%; and 4.824 MeV, 84.3%) will overlap with the (234)U doublet peak (4.722 MeV, 28.4%; and 4.775 MeV, 71.4%), if present, resulting in a combined (233+234)U multiplet. A technique for quantifying both (233)U and (234)U from alpha spectra was investigated. A series of groundwater samples were measured both by accelerator mass spectrometry (AMS) to determine (233)U/(234)U atom and activity ratios and by alpha spectrometry in order to establish a reliable (233)U estimation technique using alpha spectra. The Genie™ 2000 Alpha Analysis and Interactive Peak Fitting (IPF) software packages were used and it was found that IPF with identification of three peaks ((234)U minor, combined (234)U major and (233)U minor, and (233)U major) followed by interference correction on the combined peak and a weighted average activity calculation gave satisfactory agreement with the AMS data across the (233)U/(234)U activity ratio range (0.1-20) and (233)U activity range (2-300 mBq) investigated. Correlation between the AMS (233)U and alpha spectrometry (233)U was r(2) = 0.996 (n = 10).

  10. Measurement of Actinides in Environmental Samples at Micro-Becquerel Levels by Accelerator Mass Spectrometry

    SciTech Connect

    Brown, T A; Knezovich, J P; Marchetti, A A; Hamilton, T F

    2002-09-03

    The need for ultra-sensitive actinide measurements continues to expand in the fields of environmental stewardship, nuclear isotope forensics, radiobioassay and environmental research. We have developed a heavy isotope accelerator mass spectrometry (AMS) system at Lawrence Livermore National Laboratory's Center for Accelerator Mass Spectrometry (CAMS). The system was designed particularly for the measurement of actinide concentrations and isotopic ratios. A fast isotope switching capability has been incorporated in the system, allowing flexibility in isotope selection and for the quasi-continuous normalization to a reference isotope spike. Initially, our utilization of the system has concentrated on the measurement of Pu isotopes. Under current operating conditions, background levels equivalent to <10{sup 6} atoms are observed during routine {sup 239}Pu and {sup 240}Pu measurements. Measurements of samples containing 10{sup 13} {sup 238}U atoms demonstrate that the system provides a {sup 238}U rejection factor of >10{sup 7}. Recently, we have utilized the high dynamic range of the AMS system in measuring samples whose Pu contents ranged from <10{sup 6} (background) to >10{sup 11} Pu atoms. Measurements of known materials, combined with results from an externally organized intercomparison program, indicate that our {sup 239}Pu measurements are accurate and precise down to the {mu}Bq level ({approx}10{sup 6} atoms). The development of the heavy isotope system was undertaken with particular interest in the measurement of environmental samples, including soils, sediments, waters, air filters, tissue samples, and human urine. The high rejection of interferences, including molecular interferences, and low susceptibility to matrix components, provided by the AMS technique are of particular relevance for such complex samples. These two factors significantly reduce demands on sample preparation chemistry for Pu analyses, allowing relatively simple, cost-effective procedures

  11. Detecting and Removing Data Artifacts in Hadamard Transform Ion Mobility-Mass Spectrometry Measurements

    DOE PAGES

    Prost, Spencer A.; Crowell, Kevin L.; Baker, Erin Shammel; Ibrahim, Yehia M.; Clowers, Brian H.; Monroe, Matthew E.; Anderson, Gordon A.; Smith, Richard D.; Payne, Samuel H.

    2014-05-06

    Applying Hadamard transform multiplexing to ion mobility separations (IMS) can significantly improve the signal-to-noise ratio and throughput for IMS coupled mass spectrometry (MS) measurements by increasing the ion utilization efficiency. However, it has been determined that both fluctuations in ion intensity as well as spatial shifts in the multiplexed data lower the signal-to-noise ratios and appear as noise in downstream processing of the data. To address this problem, we have developed a novel algorithm that discovers and eliminates data artifacts. The algorithm uses knowledge of the true signal peaks derived from the encoded data and allows for both artifacts andmore » noise to be removed with high confidence, decreasing the likelihood of false identifications in subsequent data processing. The result is that IMS-MS can be applied to increase measurement sensitivity while avoiding artifacts that have previously limited its utility.« less

  12. Detecting and Removing Data Artifacts in Hadamard Transform Ion Mobility-Mass Spectrometry Measurements

    NASA Astrophysics Data System (ADS)

    Prost, Spencer A.; Crowell, Kevin L.; Baker, Erin S.; Ibrahim, Yehia M.; Clowers, Brian H.; Monroe, Matthew E.; Anderson, Gordon A.; Smith, Richard D.; Payne, Samuel H.

    2014-12-01

    Applying Hadamard transform multiplexing to ion mobility separations (IMS) can significantly improve the signal-to-noise ratio and throughput for IMS coupled mass spectrometry (MS) measurements by increasing the ion utilization efficiency. However, it has been determined that fluctuations in ion intensity as well as spatial shifts in the multiplexed data lower the signal-to-noise ratios and appear as noise in downstream processing of the data. To address this problem, we have developed a novel algorithm that discovers and eliminates data artifacts. The algorithm employs an analytical approach to identify and remove artifacts from the data, decreasing the likelihood of false identifications in subsequent data processing. Following application of the algorithm, IMS-MS measurement sensitivity is greatly increased and artifacts that previously limited the utility of applying the Hadamard transform to IMS are avoided. [Figure not available: see fulltext.

  13. Lead Slowing Down Spectrometry Analysis of Data from Measurements on Nuclear Fuel

    SciTech Connect

    Warren, Glen A.; Anderson, Kevin K.; Kulisek, Jonathan A.; Danon, Yaron; Weltz, Adam; Gavron, Victor A.; Harris, Jason; Stewart, Trevor N.

    2015-01-12

    Improved non-destructive assay of isotopic masses in used nuclear fuel would be valuable for nuclear safeguards operations associated with the transport, storage and reprocessing of used nuclear fuel. Our collaboration is examining the feasibility of using lead slowing down spectrometry techniques to assay the isotopic fissile masses in used nuclear fuel assemblies. We present the application of our analysis algorithms on measurements conducted with a lead spectrometer. The measurements involved a single fresh fuel pin and discrete 239Pu and 235U samples. We are able to describe the isotopic fissile masses with root mean square errors over seven different configurations to 6.35% for 239Pu and 2.7% for 235U over seven different configurations. Funding Source(s):

  14. Detecting and Removing Data Artifacts in Hadamard Transform Ion Mobility-Mass Spectrometry Measurements

    SciTech Connect

    Prost, Spencer A.; Crowell, Kevin L.; Baker, Erin Shammel; Ibrahim, Yehia M.; Clowers, Brian H.; Monroe, Matthew E.; Anderson, Gordon A.; Smith, Richard D.; Payne, Samuel H.

    2014-05-06

    Applying Hadamard transform multiplexing to ion mobility separations (IMS) can significantly improve the signal-to-noise ratio and throughput for IMS coupled mass spectrometry (MS) measurements by increasing the ion utilization efficiency. However, it has been determined that both fluctuations in ion intensity as well as spatial shifts in the multiplexed data lower the signal-to-noise ratios and appear as noise in downstream processing of the data. To address this problem, we have developed a novel algorithm that discovers and eliminates data artifacts. The algorithm uses knowledge of the true signal peaks derived from the encoded data and allows for both artifacts and noise to be removed with high confidence, decreasing the likelihood of false identifications in subsequent data processing. The result is that IMS-MS can be applied to increase measurement sensitivity while avoiding artifacts that have previously limited its utility.

  15. Measurements of indoor gamma radiation and radon concentrations in dwellings of Riyadh city, Saudi Arabia.

    PubMed

    Al-Saleh, Ferdoas S

    2007-07-01

    Indoor gamma radiation measurement at dwellings of Riyadh city in Saudi Arabia using TLD has been performed. Measurements were carried out from October 2004 to June 2005. The city was divided into five sectors, for four categories of bed rooms, living rooms, bathrooms and kitchens. The indoor gamma annual absorbed dose of Riyadh city is in the range from 303+/-57 to 700+/-38microGyy(-1) with an average value of 455.1+/-45microGyy(-1). The calculated corresponding annual effective dose to the adult population of the locations will vary from 212+/-40 to 490+/-27microSvy(-1) with an average value of 318.57+/-31microSvy(-1).(222)Rn concentration was measured at dwellings of Riyadh city in Saudi Arabia to estimate effective annual dose to the public from (222)Rn and its progeny. The (222)Rn concentrations were measured using CR-39 detector. The range of annual mean (222)Rn concentrations for all sites was 2-69Bqm(-3) with an average of 18.4Bqm(-3). The effective annual dose was estimated to be 0.46mSvy(-1).

  16. Investigating the Anisotropic Scintillation Response in Anthracene through Neutron, Gamma-Ray, and Muon Measurements

    NASA Astrophysics Data System (ADS)

    Schuster, Patricia; Brubaker, Erik

    2016-06-01

    This paper reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline anthracene to incident DT neutrons, DD neutrons, Cs-137 gamma rays, and, for the first time, cosmic ray muons. The neutron measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature. In similar measurements using incident gamma rays, no directional effect is evident, and any anisotropy with respect to the electron recoil direction is constrained to have a magnitude of less than a tenth of that present in the proton recoil events. Cosmic muons are measured at two directions, and no anisotropy is observed. This set of observations indicates that high dE/dx is necessary for an anisotropy to be present for a given type of scintillation event, which in turn could be used to discriminate among different hypotheses for the underlying causes of the anisotropy, which are not well understood.

  17. Investigating the anisotropic scintillation response in anthracene through neutron, gamma-ray, and muon measurements

    DOE PAGES

    Schuster, Patricia; Brubaker, Erik

    2016-05-05

    Our paper reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline anthracene to incident DT neutrons, DD neutrons, 137Cs gamma rays, and, for the first time, cosmic ray muons. Moreover, the neutron measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature. In similar measurements using incident gamma rays, no directional effect is evident, and any anisotropy with respect to the electron recoil direction is constrained to have a magnitude of less than a tenth ofmore » that present in the proton recoil events. Cosmic muons are measured at two directions, and no anisotropy is observed. Our set of observations indicates that high dE/dx is necessary for an anisotropy to be present for a given type of scintillation event, which in turn could be used to discriminate among different hypotheses for the underlying causes of the anisotropy, which are not well understood.« less

  18. Measurement of proton polarization in the d({gamma},p)n reaction

    SciTech Connect

    Geesaman, D.F.; Jackson, H.E.; Jones, C.E.

    1995-08-01

    A proposal was approved by CEBAF PAC7 to measure angular distributions of the proton polarization for the d({gamma},p)n reaction in the GeV region. This proposed measurement will test the validity of extensions of conventional nuclear-physics theories to the higher energy regime. The results of the experiment will further constrain the evidence from SLAC experiments NE8 and NE17 that asymptotic scaling was observed above a photon energy of 1.3 GeV. Photoproton polarization measurements at lower energy indicate that the magnitude of the polarization increases with energy. This is consistent with the observation that polarizations are large in high-energy processes, e.g. A{sub nn} in pp {yields} pp scattering or A{sub y} in pp {yields} {pi}{sup 0}X. However, the polarizations in hadron-hadron scattering are believed to arise from Landshoff mechanisms. The higher energy photoproton experiment will permit the first measurements of polarization for a reaction, {gamma}d {yields} pn, where there are no Landshoff terms. The experiment would make use of a polarimeter installed in either the High Resolution Spectrometer in Hall A or the Short Orbit Spectrometer in Hall C at CEBAF.

  19. Measuring kinetic isotope effects in enzyme reactions using time-resolved electrospray mass spectrometry.

    PubMed

    Liuni, Peter; Olkhov-Mitsel, Ekaterina; Orellana, Arturo; Wilson, Derek J

    2013-04-01

    Kinetic isotope effect (KIE) measurements are a powerful tool for studying enzyme mechanisms; they can provide insights into microscopic catalytic processes and even structural constraints for transition states. However, KIEs have not come into widespread use in enzymology, due in large part to the requirement for prohibitively cumbersome experimental procedures and daunting analytical frameworks. In this work, we introduce time-resolved electrospray ionization mass spectrometry (TRESI-MS) as a straightforward, precise, and inexpensive method for measuring KIEs. Neither radioisotopes nor large amounts of material are needed and kinetic measurements for isotopically "labeled" and "unlabeled" species are acquired simultaneously in a single "competitive" assay. The approach is demonstrated first using a relatively large isotope effect associated with yeast alcohol dehydrogenase (YADH) catalyzed oxidation of ethanol. The measured macroscopic KIE of 2.19 ± 0.05 is consistent with comparable measurements in the literature but cannot be interpreted in a way that provides insights into isotope effects in individual microscopic steps. To demonstrate the ability of TRESI-MS to directly measure intrinsic KIEs and to characterize the precision of the technique, we measure a much smaller (12)C/(13)C KIE associated specifically with presteady state acylation of chymotrypsin during hydrolysis of an ester substrate.

  20. Concentration of Uranium Radioisotopes in Albanian Drinking Waters Measured by Alpha Spectrometry

    NASA Astrophysics Data System (ADS)

    Bylyku, Elida; Cfarku, Florinda; Deda, Antoneta; Bode, Kozeta; Fishka, Kujtim

    2010-01-01

    Uranium is a radioactive material that is frequently found in rocks and soil. When uranium decays, it changes into different elements that are also radioactive, including radon, a gas that is known to cause a lung cancer. The main concern with uranium in drinking water is harm to the kidneys. Public water systems are required to keep uranium levels at or below 500 mBq per liter to protect against kidney damage. Such an interest is needed due to safety, regulatory compliance and disposal issue for uranium in the environment since uranium is included as an obligatory controlled radionuclide in the European Legislation (Directive 98/83 CE of Council of 03.11.1998). The aim of this work is to measure the levels of uranium in drinking and drilled well waters in Albania. At first each sample was measured for total Alpha and total Beta activity. The samples with the highest levels of total alpha activity were chosen for the determination of uranium radioisotopes by alpha spectrometry. A radiochemical procedure using extraction with TBP (Tri-Butyl-Phosphate) is used in the presence of U232 as a yield tracer. Thin sources for alpha spectrometry are prepared by electrodepositing on to stainless steel discs. The results of the U238 activity measured in the different samples, depending from their geological origin range between 0.55-13.87 mBq/l. All samples measured results under the European Directive limits for U238 (5-500 mBq/1), Dose Coefficients according to Directive 96/29 EURATOM.

  1. Neutron and gamma-ray measurements on the LANL Little Boy Comet Assembly

    SciTech Connect

    Hankins, D.E.

    1983-09-01

    We measured the neutron and gamma-ray dose rates at various distances from the Little Boy Comet Assembly at Los Alamos National Laboratory (LANL), Los Alamos, New Mexico on April 28 and 29, 1983. The distances selected varied from 350 ft to 1860 ft from the assembly, with the latter point being located at the edge of the mesa overlooking Pajarito Canyon. We varied the power levels for the various runs but we have normalized all of them to a single power-level. We also made corrections for the variations in the power-level indicators of the assembly using data provided by LANL.

  2. System of Programmed Modules for Measuring Photographs with a Gamma-Telescope

    NASA Technical Reports Server (NTRS)

    Averin, S. A.; Veselova, G. V.; Navasardyan, G. V.

    1978-01-01

    Physical experiments using tracking cameras resulted in hundreds of thousands of stereo photographs of events being received. To process such a large volume of information, automatic and semiautomatic measuring systems are required. At the Institute of Space Research of the Academy of Science of the USSR, a system for processing film information from the spark gamma-telescope was developed. The system is based on a BPS-75 projector in line with the minicomputer Elektronika 1001. The report describes this system. The various computer programs available to the operators are discussed.

  3. Actinide Measurements by Accelerator Mass Spectrometry at Lawrence Livermore National Laboratory

    SciTech Connect

    Brown, T A; Marchetti, A A; Martinelli, R E; Cox, C C; Knezovich, J P; Hamilton, T F

    2003-09-25

    We report on the development of an accelerator mass spectrometry (AMS) system for the measurement of actinides at Lawrence Livermore National Laboratory. This AMS system is centered on a recently completed heavy isotope beam line that was designed particularly for high sensitivity, robust, high-throughput measurements of actinide concentrations and isotopic ratios. A fast isotope switching capability has been incorporated in the system, allowing flexibility in isotope selection and for the quasi-continuous normalization to a reference isotope spike. Initially, our utilization of the heavy isotope system has concentrated on the measurement of Pu isotopes. Under current operating conditions, background levels equivalent to {approx}1 x 10{sup 5} atoms are observed during routine {sup 239}Pu and {sup 240}Pu measurements. Measurements of samples containing {approx}10{sup 13} {sup 238}U atoms demonstrate that the system provides a {sup 238}U rejection factor during {sup 239}Pu measurements of {approx}10{sup 7}. Measurements of known materials, combined with results from an externally organized inter-comparison program, indicate that our {sup 239}Pu measurements are accurate and precise down to the {micro}Bq level ({approx}10{sup 6} atoms). Recently, we have investigated the performance of our heavy isotope AMS system in measurements of {sup 237}Np and {sup 236}U. Results of these investigations are discussed. The sensitivity shown by our Pu measurements, combined with the high throughput and interference rejection capabilities of our AMS system, demonstrate that AMS can provide a rapid and cost-effective measurement technique for actinides in a wide variety of studies.

  4. Hydrogen measurement during steam oxidation using coupled thermogravimetric analysis and quadrupole mass spectrometry

    DOE PAGES

    Parkison, Adam J.; Nelson, Andrew Thomas

    2016-01-11

    An analytical technique is presented with the goal of measuring reaction kinetics during steam oxidation reactions for three cases in which obtaining kinetics information often requires a prohibitive amount of time and cost. The technique presented relies on coupling thermogravimetric analysis (TGA) with a quantitative hydrogen measurement technique using quadrupole mass spectrometry (QMS). The first case considered is in differentiating between the kinetics of steam oxidation reactions and those for simultaneously reacting gaseous impurities such as nitrogen or oxygen. The second case allows one to independently measure the kinetics of oxide and hydride formation for systems in which both ofmore » these reactions are known to take place during steam oxidation. The third case deals with measuring the kinetics of formation for competing volatile and non-volatile oxides during certain steam oxidation reactions. In order to meet the requirements of the coupled technique, a methodology is presented which attempts to provide quantitative measurement of hydrogen generation using QMS in the presence of an interfering fragmentation species, namely water vapor. This is achieved such that all calibrations and corrections are performed during the TGA baseline and steam oxidation programs, making system operation virtually identical to standard TGA. Benchmarking results showed a relative error in hydrogen measurement of 5.7–8.4% following the application of a correction factor. Lastly, suggestions are made for possible improvements to the presented technique so that it may be better applied to the three cases presented.« less

  5. LAFARA: a new underground laboratory in the French Pyrénées for ultra low-level gamma-ray spectrometry.

    PubMed

    van Beek, P; Souhaut, M; Lansard, B; Bourquin, M; Reyss, J-L; von Ballmoos, P; Jean, P

    2013-02-01

    We describe a new underground laboratory, namely LAFARA (for "LAboratoire de mesure des FAibles RAdioactivités"), that was recently created in the French Pyrénées. This laboratory is primarily designed to analyze environmental samples that display low radioactivity levels using gamma-ray spectrometry. Two high-purity germanium detectors were placed under 85 m of rock (ca. 215 m water equivalent) in the tunnel of Ferrières (Ariège, France). The background is thus reduced by a factor of ∼20 in comparison to above-ground laboratories. Both detectors are fully equipped so that the samples can be analyzed in an automatic mode without requiring permanent presence of a technician in the laboratory. Auto-samplers (twenty positions) and systems to fill liquid nitrogen automatically provide one month of autonomy to the spectrometers. The LAFARA facility allows us to develop new applications in the field of environmental sciences based on the use of natural radionuclides present at low levels in the environment. As an illustration, we present two of these applications: i) dating of marine sediments using the decay of (226)Ra in sedimentary barite (BaSO(4)), ii) determination of (227)Ac ((231)Pa) activities in marine sediment cores.

  6. LAFARA: a new underground laboratory in the French Pyrénées for ultra low-level gamma-ray spectrometry.

    PubMed

    van Beek, P; Souhaut, M; Lansard, B; Bourquin, M; Reyss, J-L; von Ballmoos, P; Jean, P

    2013-02-01

    We describe a new underground laboratory, namely LAFARA (for "LAboratoire de mesure des FAibles RAdioactivités"), that was recently created in the French Pyrénées. This laboratory is primarily designed to analyze environmental samples that display low radioactivity levels using gamma-ray spectrometry. Two high-purity germanium detectors were placed under 85 m of rock (ca. 215 m water equivalent) in the tunnel of Ferrières (Ariège, France). The background is thus reduced by a factor of ∼20 in comparison to above-ground laboratories. Both detectors are fully equipped so that the samples can be analyzed in an automatic mode without requiring permanent presence of a technician in the laboratory. Auto-samplers (twenty positions) and systems to fill liquid nitrogen automatically provide one month of autonomy to the spectrometers. The LAFARA facility allows us to develop new applications in the field of environmental sciences based on the use of natural radionuclides present at low levels in the environment. As an illustration, we present two of these applications: i) dating of marine sediments using the decay of (226)Ra in sedimentary barite (BaSO(4)), ii) determination of (227)Ac ((231)Pa) activities in marine sediment cores. PMID:23164692

  7. Systematic indoor radon and gamma-ray measurements in Slovenian schools

    SciTech Connect

    Vaupotic, J.; Sikovec, M.; Kobal, I.

    2000-05-01

    During the winter months of 1992/93 and 1993/94, instantaneous indoor radon concentrations and gamma dose rates were measured in 890 schools in Slovenia attended in total by about 280,000 pupils. Under closed conditions, the room to be surveyed was closed for more than 12 h prior to sampling, the air was sampled into alpha scintillation cells with a volume of 700 cm{sup 3}, and alpha activity was measured. An arithmetic mean of 168 Bq m{sup {minus}3} and a geometric mean of 82 Bq m{sup {minus}3} were obtained. In 67% of schools, indoor radon concentrations were below 100 Bq m{sup {minus}3}, and in 8.7% (77 schools with about 16,000 pupils) they exceeded 400 Bq m{sup {minus}3}, which is the proposed Slovene action level. In the majority of cases, radon concentrations were high due to the geological characteristics of the ground. Approximately 70% of schools with high radon levels were found in the Karst region. Gamma dose rates were measured using a portable scintillation counter. An arithmetic mean of 102 nGy h{sup {minus}1} and a geometric mean of 95 nGy h{sup {minus}1} were obtained. No extraordinarily high values were recorded.

  8. Bioactive compounds of fourth generation gamma-irradiated Typhoniumflagelliforme Lodd. mutants based on gas chromatography-mass spectrometry

    NASA Astrophysics Data System (ADS)

    Sianipar, N. F.; Purnamaningsih, R.; Rosaria

    2016-08-01

    Rodent tuber (Typhonium flagelliforme Lodd.) is an Indonesian anticancer medicinal plant. The natural genetic diversity of rodent tuber is low due to vegetative propagation. Plant's genetic diversity has to be increased for obtaining clones which contain a high amount of anticancer compounds. In vitro calli were irradiated with 6 Gy of gamma ray to produce in vitro mutant plantlets. Mutant plantlets were acclimated and propagated in a greenhouse. This research was aimed to identify the chemical compounds in the leaves and tubers ofthe fourth generation of rodent tuber's vegetative mutant clones (MV4) and control plantsby using GC- MS method. Leaves and tubers of MV4 each contained 2 and 5 anticancer compounds which quantities were higher compared to control plants. MV4 leaves contained 5 new anticancer compounds while its tubers contained 3 new anticancer compounds which were not found in control. The new anticancer compounds in leaves were hexadecanoic acid, stigmast-5-en-3-ol, ergost-5-en-3-ol, farnesol isomer a, and oleic acid while the new anticancer compounds in tubers were alpha tocopherol, ergost-5-en-3-ol, and beta-elemene. Rodent tuber mutant clones are very potential to be developed into anticancer drugs.

  9. Evidence for the decay Bs0-->Ds(*)Ds(*) and a measurement of DeltaGammasCP/Gammas.

    PubMed

    Abazov, V M; Abbott, B; Abolins, M; Acharya, B S; Adams, M; Adams, T; Aguilo, E; Ahsan, M; Alexeev, G D; Alkhazov, G; Alton, A; Alverson, G; Alves, G A; Anastasoaie, M; Ancu, L S; Andeen, T; Andrieu, B; Anzelc, M S; Aoki, M; Arnoud, Y; Arov, M; Arthaud, M; Askew, A; Asman, B; Assis Jesus, A C S; Atramentov, O; Avila, C; Badaud, F; Bagby, L; Baldin, B; Bandurin, D V; Banerjee, P; Banerjee, S; Barberis, E; Barfuss, A-F; Bargassa, P; Baringer, P; Barreto, J; Bartlett, J F; Bassler, U; Bauer, D; Beale, S; Bean, A; Begalli, M; Begel, M; Belanger-Champagne, C; Bellantoni, L; Bellavance, A; Benitez, J A; Beri, S B; Bernardi, G; Bernhard, R; Bertram, I; Besançon, M; Beuselinck, R; Bezzubov, V A; Bhat, P C; Bhatnagar, V; Blazey, G; Blekman, F; Blessing, S; Bloom, K; Boehnlein, A; Boline, D; Bolton, T A; Boos, E E; Borissov, G; Bose, T; Brandt, A; Brock, R; Brooijmans, G; Bross, A; Brown, D; Bu, X B; Buchanan, N J; Buchholz, D; Buehler, M; Buescher, V; Bunichev, V; Burdin, S; Burnett, T H; Buszello, C P; Calfayan, P; Calvet, S; Cammin, J; Carrasco-Lizarraga, M A; Carrera, E; Carvalho, W; Casey, B C K; Castilla-Valdez, H; Chakrabarti, S; Chakraborty, D; Chan, K M; Chandra, A; Cheu, E; Cho, D K; Choi, S; Choudhary, B; Christofek, L; Christoudias, T; Cihangir, S; Claes, D; Clutter, J; Cooke, M; Cooper, W E; Corcoran, M; Couderc, F; Cousinou, M-C; Crépé-Renaudin, S; Cuplov, V; Cutts, D; Cwiok, M; da Motta, H; Das, A; Davies, G; De, K; de Jong, S J; De La Cruz-Burelo, E; De Oliveira Martins, C; DeVaughan, K; Déliot, F; Demarteau, M; Demina, R; Denisov, D; Denisov, S P; Desai, S; Diehl, H T; Diesburg, M; Dominguez, A; Dorland, T; Dubey, A; Dudko, L V; Duflot, L; Dugad, S R; Duggan, D; Duperrin, A; Dutt, S; Dyer, J; Dyshkant, A; Eads, M; Edmunds, D; Ellison, J; Elvira, V D; Enari, Y; Eno, S; Ermolov, P; Evans, H; Evdokimov, A; Evdokimov, V N; Ferapontov, A V; Ferbel, T; Fiedler, F; Filthaut, F; Fisher, W; Fisk, H E; Fortner, M; Fox, H; Fu, S; Fuess, S; Gadfort, T; Galea, C F; Garcia, C; Garcia-Bellido, A; Gavrilov, V; Gay, P; Geist, W; Geng, W; Gerber, C E; Gershtein, Y; Gillberg, D; Ginther, G; Gómez, B; Goussiou, A; Grannis, P D; Greenlee, H; Greenwood, Z D; Gregores, E M; Grenier, G; Gris, Ph; Grivaz, J-F; Grohsjean, A; Grünendahl, S; Grünewald, M W; Guo, F; Guo, J; Gutierrez, G; Gutierrez, P; Haas, A; Hadley, N J; Haefner, P; Hagopian, S; Haley, J; Hall, I; Hall, R E; Han, L; Harder, K; Harel, A; Hauptman, J M; Hays, J; Hebbeker, T; Hedin, D; Hegeman, J G; Heinson, A P; Heintz, U; Hensel, C; Herner, K; Hesketh, G; Hildreth, M D; Hirosky, R; Hoang, T; Hobbs, J D; Hoeneisen, B; Hohlfeld, M; Hossain, S; Houben, P; Hu, Y; Hubacek, Z; Hynek, V; Iashvili, I; Illingworth, R; Ito, A S; Jabeen, S; Jaffré, M; Jain, S; Jakobs, K; Jarvis, C; Jesik, R; Johns, K; Johnson, C; Johnson, M; Johnston, D; Jonckheere, A; Jonsson, P; Juste, A; Kajfasz, E; Karmanov, D; Kasper, P A; Katsanos, I; Kaushik, V; Kehoe, R; Kermiche, S; Khalatyan, N; Khanov, A; Kharchilava, A; Kharzheev, Y N; Khatidze, D; Kim, T J; Kirby, M H; Kirsch, M; Klima, B; Kohli, J M; Konrath, J-P; Kozelov, A V; Kraus, J; Kuhl, T; Kumar, A; Kupco, A; Kurca, T; Kuzmin, V A; Kvita, J; Lacroix, F; Lam, D; Lammers, S; Landsberg, G; Lebrun, P; Lee, W M; Leflat, A; Lellouch, J; Li, J; Li, L; Li, Q Z; Lietti, S M; Lim, J K; Lima, J G R; Lincoln, D; Linnemann, J; Lipaev, V V; Lipton, R; Liu, Y; Liu, Z; Lobodenko, A; Lokajicek, M; Love, P; Lubatti, H J; Luna-Garcia, R; Lyon, A L; Maciel, A K A; Mackin, D; Madaras, R J; Mättig, P; Magerkurth, A; Mal, P K; Malbouisson, H B; Malik, S; Malyshev, V L; Maravin, Y; Martin, B; McCarthy, R; Meijer, M M; Melnitchouk, A; Mendoza, L; Mercadante, P G; Merkin, M; Merritt, K W; Meyer, A; Meyer, J; Mitrevski, J; Mommsen, R K; Mondal, N K; Moore, R W; Moulik, T; Muanza, G S; Mulhearn, M; Mundal, O; Mundim, L; Nagy, E; Naimuddin, M; Narain, M; Neal, H A; Negret, J P; Neustroev, P; Nilsen, H; Nogima, H; Novaes, S F; Nunnemann, T; O'Neil, D C; Obrant, G; Ochando, C; Onoprienko, D; Oshima, N; Osman, N; Osta, J; Otec, R; Otero Y Garzón, G J; Owen, M; Padley, P; Pangilinan, M; Parashar, N; Park, S-J; Park, S K; Parsons, J; Partridge, R; Parua, N; Patwa, A; Pawloski, G; Penning, B; Perfilov, M; Peters, K; Peters, Y; Pétroff, P; Petteni, M; Piegaia, R; Piper, J; Pleier, M-A; Podesta-Lerma, P L M; Podstavkov, V M; Pogorelov, Y; Pol, M-E; Polozov, P; Pope, B G; Popov, A V; Potter, C; Prado da Silva, W L; Prosper, H B; Protopopescu, S; Qian, J; Quadt, A; Quinn, B; Rakitine, A; Rangel, M S; Ranjan, K; Ratoff, P N; Renkel, P; Rich, P; Rijssenbeek, M; Ripp-Baudot, I; Rizatdinova, F; Robinson, S; Rodrigues, R F; Rominsky, M; Royon, C; Rubinov, P; Ruchti, R; Safronov, G; Sajot, G; Sánchez-Hernández, A; Sanders, M P; Sanghi, B; Savage, G; Sawyer, L; Scanlon, T; Schaile, D; Schamberger, R D; Scheglov, Y; Schellman, H; Schliephake, T; Schlobohm, S; Schwanenberger, C; Schwartzman, A; Schwienhorst, R; Sekaric, J; Severini, H; Shabalina, E; Shamim, M; Shary, V; Shchukin, A A; Shivpuri, R K; Siccardi, V; Simak, V; Sirotenko, V; Skubic, P; Slattery, P; Smirnov, D; Snow, G R; Snow, J; Snyder, S; Söldner-Rembold, S; Sonnenschein, L; Sopczak, A; Sosebee, M; Soustruznik, K; Spurlock, B; Stark, J; Stolin, V; Stoyanova, D A; Strandberg, J; Strandberg, S; Strang, M A; Strauss, E; Strauss, M; Ströhmer, R; Strom, D; Stutte, L; Sumowidagdo, S; Svoisky, P; Sznajder, A; Tanasijczuk, A; Taylor, W; Tiller, B; Tissandier, F; Titov, M; Tokmenin, V V; Torchiani, I; Tsybychev, D; Tuchming, B; Tully, C; Tuts, P M; Unalan, R; Uvarov, L; Uvarov, S; Uzunyan, S; Vachon, B; van den Berg, P J; Van Kooten, R; van Leeuwen, W M; Varelas, N; Varnes, E W; Vasilyev, I A; Verdier, P; Vertogradov, L S; Verzocchi, M; Vilanova, D; Villeneuve-Seguier, F; Vint, P; Vokac, P; Voutilainen, M; Wagner, R; Wahl, H D; Wang, M H L S; Warchol, J; Watts, G; Wayne, M; Weber, G; Weber, M; Welty-Rieger, L; Wenger, A; Wermes, N; Wetstein, M; White, A; Wicke, D; Williams, M R J; Wilson, G W; Wimpenny, S J; Wobisch, M; Wood, D R; Wyatt, T R; Xie, Y; Xu, C; Yacoob, S; Yamada, R; Yang, W-C; Yasuda, T; Yatsunenko, Y A; Yin, H; Yip, K; Yoo, H D; Youn, S W; Yu, J; Zeitnitz, C; Zelitch, S; Zhao, T; Zhou, B; Zhu, J; Zielinski, M; Zieminska, D; Zieminski, A; Zivkovic, L; Zutshi, V; Zverev, E G

    2009-03-01

    We search for the semi-inclusive process Bs0-->Ds(*)Ds(*) using 2.8 fb(-1) of pp collisions at sqrt[s]=1.96 TeV recorded by the D0 detector operating at the Fermilab Tevatron Collider. We observe 26.6+/-8.4 signal events with a significance above background of 3.2 standard deviations yielding a branching ratio of B(Bs0-->Ds(*)Ds(*))=0.035+/-0.010(stat.)+/-0.011(syst.). Under certain theoretical assumptions, these double-charm final states saturate CP-even eigenstates in the Bs0 decays resulting in a width difference of DeltaGammasCP/Gammas=0.072+/-0.021(stat.)+/-0.022(syst.). PMID:19392506

  10. MULTI-POLLUTANT CONCENTRATION MEASUREMENTS AROUND A CONCENTRATED SWINE PRODUCTION FACILITY USING OPEN-PATH FTIR SPECTROMETRY

    EPA Science Inventory

    Open-path Fourier transform infrared (OP/FTIR) spectrometry was used to measure the concentrations of ammonia, methane, and other atmospheric gasses around an integrated industrial swine production facility in eastern North Carolina. Several single-path measurements were made ove...

  11. Development of array-type prompt gamma measurement system for in vivo range verification in proton therapy

    SciTech Connect

    Min, Chul Hee; Lee, Han Rim; Kim, Chan Hyeong; Lee, Se Byeong

    2012-04-15

    Purpose: In vivo range verification is one of the most important parts of proton therapy to fully utilize its benefits delivering high radiation dose to tumor, while sparing the normal tissue with the so-called Bragg peak. Currently, however, range verification method is not used in clinics. The purpose of the present study is to optimize and evaluate the configuration of an array-type prompt gamma measurement system on determining distal dose edge for in vivo range verification of proton therapy. Methods: To effectively measure the prompt gammas against the background gammas, the Monte Carlo simulations with the MCNPX code were employed in optimizing the configuration of the measurement system, and the Monte Carlo method was also used to understand the effect of the background gammas, mainly neutron capture gammas, in the measured gamma distribution. To reduce the effect of the background gammas, the optimized energy window of 4-10 MeV in measuring the prompt gammas was employed. A parameterized source was used to maximize computation speed in the optimization study. A simplified test measurement system, using only one detector moving from one measurement location to the next, was constructed and applied to therapeutic proton beams of 80-220 MeV. For accurate determination of the distal dose edge, the sigmoidal curve-fitting method was applied to the measured distributions of the prompt gammas, and then, the location of the half-value between the maximum and minimum value in the curve-fitting was determined as the distal dose edge and compared with the beam range assessed by the proton dose distribution. Results: The parameterized source term employed in optimization process improved the calculation speed by up to {approx}300 times. The optimization study indicates that an array-type measurement system with 3, 2, 2, and 150 mm for scintillator thickness, slit width, septal thickness, and slit length, respectively, can effectively measure the prompt gamma

  12. Time-delay spectrometry measurement of magnitude and phase of hydrophone response.

    PubMed

    Wear, Keith A; Gammell, Paul M; Maruvada, Subha; Liu, Yunbo; Harris, Gerald R

    2011-11-01

    A method based on time-delay spectrometry (TDS) was developed for measuring both magnitude and phase response of a hydrophone. The method was tested on several types of hydrophones used in medical ultrasound exposimetry over the range from 5 to 18 MHz. These included polyvinylidene fluoride (PVDF) spot-poled membrane, needle, and capsule designs. One needle hydrophone was designed for high-intensity focused ultrasound (HIFU) applications. The average reproducibility (after repositioning the hydrophone) of the phase measurement was 2.4°. The minimum-phase model, which implies that the phase response is equal to the inverse Hilbert transform of the natural logarithm of the magnitude response, was tested with TDS hydrophone data. Direct TDS-based measurements of hydrophone phase responses agreed well with calculations based on the minimum-phase model, with rms differences of 1.76° (PVDF spot-poled membrane hydrophone), 3.10° (PVDF capsule hydrophone), 3.43° (PVDF needle hydrophone), and 3.36° (ceramic needle hydrophone) over the range from 5 to 18 MHz. Therefore, phase responses for several types of hydrophones may be inferred from measurements of their magnitude responses. Calculation of phase response based on magnitude response using the minimumphase model is a relatively simple and practical alternative to direct measurement of phase. PMID:22083766

  13. Characterization of uranium bearing material using x-ray fluorescence and direct gamma-rays measurement techniques

    NASA Astrophysics Data System (ADS)

    Mujaini, M.; Chankow, N.; Yusoff, M. Z.; Hamid, N. A.

    2016-01-01

    Uranium ore can be easily detected due to various gamma-ray energies emitted from uranium daughters particularly from 238U daughters such as 214Bi, 214Pb and 226Ra. After uranium is extracted from uranium ore, only low energy gamma-rays emitted from 235U may be detected if the detector is placed in close contact to the specimen. In this research, identification and characterization of uranium bearing materials is experimentally investigated using direct measurement of gamma-rays from 235U in combination with the x-ray fluorescence (XRF) technique. Measurement of gamma-rays can be conducted by using high purity germanium (HPGe) detector or cadmium telluride (CdTe) detector while a 57Coradioisotope-excited XRF spectrometer using CdTe detector is used for elemental analysis. The proposed technique was tested with various uranium bearing specimens containing natural, depleted and enriched uranium in both metallic and powder forms.

  14. Measuring the activity of a {sup 51}Cr neutrino source based on the gamma-radiation spectrum

    SciTech Connect

    Gorbachev, V. V. Gavrin, V. N.; Ibragimova, T. V.; Kalikhov, A. V.; Malyshkin, Yu. M.; Shikhin, A. A.

    2015-12-15

    A technique for the measurement of activities of intense β sources by measuring the continuous gamma-radiation (internal bremsstrahlung) spectra is developed. A method for reconstructing the spectrum recorded by a germanium semiconductor detector is described. A method for the absolute measurement of the internal bremsstrahlung spectrum of {sup 51}Cr is presented.

  15. Isotopic abundance measurements on solid nuclear-type samples by glow discharge mass spectrometry.

    PubMed

    Betti, M; Rasmussen, G; Koch, L

    1996-07-01

    A double-focusing Glow Discharge Mass Spectrometer (GDMS) installed in a glovebox for nuclear sample screening has been employed for isotopic measurements. Isotopic compositions of zirconium, silicon, lithium, boron, uranium and plutonium which are elements of nuclear concern have been determined. Interferences arising from the matrix sample and the discharge gas (Ar) for each of these elements are discussed. The GDMS results are compared with those from Thermal Ionization Mass Spectrometry (TIMS). For boron and lithium at microg/g-ng/g levels, the two methods gave results in good agreement. In samples containing uranium the isotopic composition obtained by GDMS was in agreement with those from TIMS independently of the enrichment. Attempts for the determination of plutonium isotopic composition were also made. In this case, due to the interferences of uranium at mass 238 and americium at mass 241, the GDMS raw data are complementary with those values obtained from physical non-destructive techniques.

  16. Measurement of the PPN Parameter (gamma) with radio signals from the Cassini Spacecraft at X- and Ka-Bands

    NASA Technical Reports Server (NTRS)

    Anderson, John D.; Lau, Eunice L.; Giampieri, Giacomo

    2005-01-01

    Radio Doppler data from the Cassini spacecraft during its solar conjunction in June 2002 can be used to measure the bending of light by solar gravitation. In terms of the standard post-Newtonian parameter (gamma), we find that (gamma) - 1 = (-1.3 +/- 5.2)x10^-5 in agreement with the theory of General Relativity. This result implies that the parameter (omega) in the Brans-Dicke theory is greater than 9000 at a 95% confidence level.

  17. Measuring Hordein (Gluten) in Beer – A Comparison of ELISA and Mass Spectrometry

    PubMed Central

    Blundell, Malcolm J.; Goswami, Hareshwar P.; Howitt, Crispin A.

    2013-01-01

    Background Subjects suffering from coeliac disease, gluten allergy/intolerance must adopt a lifelong avoidance of gluten. Beer contains trace levels of hordeins (gluten) which are too high to be safely consumed by most coeliacs. Accurate measurement of trace hordeins by ELISA is problematic. Methods We have compared hordein levels in sixty beers, by sandwich ELISA, with the level determined using multiple reaction monitoring mass spectrometry (MRM-MS). Results Hordein levels measured by ELISA varied by four orders of magnitude, from zero (for known gluten-free beers) to 47,000 µg/mL (ppm; for a wheat-based beer). Half the commercial gluten-free beers were free of hordein by MS and ELISA. Two gluten-free and two low-gluten beers had zero ELISA readings, but contained significant hordein levels (p<0.05), or near average (60–140%) hordein levels, by MS, respectively. Six beers gave false negatives, with zero ELISA readings but near average hordein content by MS. Approximately 20% of commercial beers had ELISA readings less than 1 ppm, but a near average hordein content by MS. Several barley beers also contained undeclared wheat proteins. Conclusions ELISA results did not correlate with the relative content of hordein peptides determined by MS, with all barley based beers containing hordein. We suggest that mass spectrometry is more reliable than ELISA, as ELISA enumerates only the concentration of particular amino-acid epitopes; this may vary between different hordeins and may not be related to the absolute hordein concentration. MS quantification is undertaken using peptides that are specific and unique, enabling the quantification of individual hordein isoforms. This outlines the problem of relying solely on ELISA determination of gluten in beverages such as beer and highlights the need for the development of new sensitive and selective quantitative assay such as MS. PMID:23509606

  18. Biomedical applications of accelerator mass spectrometry-isotope measurements at the level of the atom.

    PubMed

    Barker, J; Garner, R C

    1999-01-01

    Accelerator mass spectrometry (AMS) is a nuclear physics technique developed about twenty years ago, that uses the high energy (several MeV) of a tandem Van de Graaff accelerator to measure very small quantities of rare and long-lived isotopes. Elements that are of interest in biomedicine and environmental sciences can be measured, often to parts per quadrillion sensitivity, i.e. zeptomole to attomole levels (10(-21)-10(-18) mole) from milligram samples. This is several orders of magnitude lower than that achievable by conventional decay counting techniques, such as liquid scintillation counting (LSC). AMS was first applied to geochemical, climatological and archaeological areas, such as for radiocarbon dating (Shroud of Turin), but more recently this technology has been used for bioanalytical applications. In this sphere, most work has been conducted using aluminium, calcium and carbon isotopes. The latter is of special interest in drug metabolism studies, where a Phase 1 adsorption, distribution, metabolism and excretion (ADME) study can be conducted using only 10 nanoCurie (37 Bq or ca. 0.9 microSv) amounts or less of 14C-labelled drugs. In the UK, these amounts of radioactivity are below those necessary to request specific regulatory approval from the Department of Health's Administration of Radioactive Substances Advisory Committee (ARSAC), thus saving on valuable development time and resources. In addition, the disposal of these amounts is much less an environmental issue than that associated with microCurie quantities, which are currently used. Also, AMS should bring an opportunity to conduct "first into man" studies without the need for widespread use of animals. Centre for Biomedical Accelerator Mass Spectrometry (CBAMS) Ltd. is the first fully commercial company in the world to offer analytical services using AMS. With its high throughput and relatively low costs per sample analysis, AMS should be of great benefit to the pharmaceutical and biotechnology

  19. Hybrid Quadrupole-Orbitrap mass spectrometry for quantitative measurement of quorum sensing inhibition.

    PubMed

    Todd, Daniel A; Zich, David B; Ettefagh, Keivan A; Kavanaugh, Jeffrey S; Horswill, Alexander R; Cech, Nadja B

    2016-08-01

    Drug resistant bacterial infections cause significant morbidity and mortality worldwide, and new strategies are needed for the treatment of these infections. The anti-virulence approach, which targets non-essential virulence factors in bacteria, has been proposed as one way to combat the problem of antibiotic resistance. Virulence in methicillin-resistant Staphylococcus aureus (MRSA) and many other Gram-positive bacterial pathogens is controlled by the quorum sensing system. Thus, there is excellent therapeutic potential for compounds that target this system. With this project, we have developed and validated a novel approach for measuring quorum sensing inhibition in vitro. Ultraperformance liquid chromatography coupled to mass spectrometry (UPLC-MS) was employed to directly measure one of the important outputs of the quorum sensing system in MRSA, auto-inducing peptide I (AIP I) in bacterial cultures. The method for AIP detection was validated and demonstrated limits of detection and quantification of range of 0.0035μM and 0.10μM, respectively. It was shown that the known quorum sensing inhibitor ambuic acid inhibited AIP I production by a clinically relevant strain of MRSA, with an IC50 value of 2.6±0.2μM. The new method performed similarly to previously published methods using GFP reporter assays, but has the advantage of being applicable without the need for engineering of a reporter strain. Additionally, the mass spectrometry-based method could be applicable in situations where interference by the inhibitor prevents the application of fluorescence-based methods. PMID:27237773

  20. Cluster Ion Spectrometry (CIS) data quality indexes as a support for analysing magnetospheric measurements

    NASA Astrophysics Data System (ADS)

    Dandouras, Iannis; Barthe, Alain; Brunato, Sylvain; Rème, Henri; Laakso, Harri

    2016-04-01

    The Cluster Science Archive (CSA) aims at preserving the complete set of the measurements collected by the four Cluster spacecraft, so that they are usable in the long-term by the world-wide scientific community as well as by the instrument teams. This implies that the instrument data, properly calibrated, are filed together with the descriptive and documentary elements making it possible to select and interpret them. The CIS (Cluster Ion Spectrometry) experiment is a comprehensive ionic plasma spectrometry package onboard the Cluster spacecraft, capable of obtaining full three-dimensional ion distributions (about 0 to 40 keV/e) with a time resolution of one spacecraft spin (4 sec) and with mass-per-charge composition determination. For the archival of the CIS data a multi-level approach has been adopted. The CSA archival includes processed raw data, moments of the ion distribution functions, and calibrated high-resolution data in a variety of physical units. The latter are 3-D ion distribution functions, 2-D pitch-angle distributions and 1-D omni-directional fluxes. The CIS data archive includes also experiment documentation, graphical products for browsing through the data, data caveats and data quality indexes. The later constitute a novel product, which has been prepared in order to help the user asses the quality of the data acquired in different magnetospheric regions and during various operational modes. It provides information on which are in each case the issues that can affect the data quality, which are the data products affected, and gives a simple quantitative measurement of the severity of these issues. The principle of the CIS data quality indexes will be described and the various issues, that can under some conditions affect the data quality and are thus taken into account in generating the data quality indexes, will be discussed.

  1. Hybrid Quadrupole-Orbitrap mass spectrometry for quantitative measurement of quorum sensing inhibition.

    PubMed

    Todd, Daniel A; Zich, David B; Ettefagh, Keivan A; Kavanaugh, Jeffrey S; Horswill, Alexander R; Cech, Nadja B

    2016-08-01

    Drug resistant bacterial infections cause significant morbidity and mortality worldwide, and new strategies are needed for the treatment of these infections. The anti-virulence approach, which targets non-essential virulence factors in bacteria, has been proposed as one way to combat the problem of antibiotic resistance. Virulence in methicillin-resistant Staphylococcus aureus (MRSA) and many other Gram-positive bacterial pathogens is controlled by the quorum sensing system. Thus, there is excellent therapeutic potential for compounds that target this system. With this project, we have developed and validated a novel approach for measuring quorum sensing inhibition in vitro. Ultraperformance liquid chromatography coupled to mass spectrometry (UPLC-MS) was employed to directly measure one of the important outputs of the quorum sensing system in MRSA, auto-inducing peptide I (AIP I) in bacterial cultures. The method for AIP detection was validated and demonstrated limits of detection and quantification of range of 0.0035μM and 0.10μM, respectively. It was shown that the known quorum sensing inhibitor ambuic acid inhibited AIP I production by a clinically relevant strain of MRSA, with an IC50 value of 2.6±0.2μM. The new method performed similarly to previously published methods using GFP reporter assays, but has the advantage of being applicable without the need for engineering of a reporter strain. Additionally, the mass spectrometry-based method could be applicable in situations where interference by the inhibitor prevents the application of fluorescence-based methods.

  2. Airborne gamma radiation measurements of soil moisture during FIFE: Activities and results

    NASA Technical Reports Server (NTRS)

    Peck, Eugene L.

    1992-01-01

    Soil moisture measurements were obtained during the summer of 1987 and 1989 near Manhattan, Kansas, using the National Weather Service (NWS) airborne gamma radiation system. A network of 24 flight lines were established over the research area. Airborne surveys were flown daily during two intensive field campaigns. The data collected was sufficient to modify the NWS standard operational method for estimating soil moisture for the Field Experiment (FIFE) flight lines. The average root mean square error of the soil moisture estimates for shorter FIFE flight lines was found to be 2.5 percent, compared with a reported value of 3.9 percent for NWS flight lines. Techniques were developed to compute soil moisture estimates for portions of the flight lines. Results of comparisons of the airborne gamma radiation soil moisture estimates with those obtained using the NASA Pushbroom Microwave Radiation (PBMR) system and hydrological model are presented. The airborne soil moisture measurements, and real averages computed using all remotely sensed and ground data, have been in support of the research of the many FIFE investigators whose overall goal was the upscale integration of models and the application of satellite remote sensing.

  3. Thermodynamic Measurements of Alloys and Compounds by Double Knudsen Cell Mass Spectrometry and Their Application to Materials Processing

    PubMed Central

    Sasaki, Hideaki; Kobashi, Yoshifumi; Nagai, Takashi; Maeda, Masafumi

    2014-01-01

    For the development and optimization of materials processing a collection of thermodynamic information concerning substances that participate in the reactions is important. One fundamental way to obtain such information is to measure the vapor pressure of gas species under conditions where they are in equilibrium with the condensed phases. Over the past 60 years Knudsen cell mass spectrometry has been used to identify and quantitatively determine gas species at high temperatures. This article describes thermodynamic foundation and examples of measurements in order to demonstrate the use of mass spectrometry focusing on the field of process metallurgy and recycling processes. PMID:26819884

  4. Thermodynamic Measurements of Alloys and Compounds by Double Knudsen Cell Mass Spectrometry and Their Application to Materials Processing.

    PubMed

    Sasaki, Hideaki; Kobashi, Yoshifumi; Nagai, Takashi; Maeda, Masafumi

    2014-01-01

    For the development and optimization of materials processing a collection of thermodynamic information concerning substances that participate in the reactions is important. One fundamental way to obtain such information is to measure the vapor pressure of gas species under conditions where they are in equilibrium with the condensed phases. Over the past 60 years Knudsen cell mass spectrometry has been used to identify and quantitatively determine gas species at high temperatures. This article describes thermodynamic foundation and examples of measurements in order to demonstrate the use of mass spectrometry focusing on the field of process metallurgy and recycling processes.

  5. Thermodynamic Measurements of Alloys and Compounds by Double Knudsen Cell Mass Spectrometry and Their Application to Materials Processing.

    PubMed

    Sasaki, Hideaki; Kobashi, Yoshifumi; Nagai, Takashi; Maeda, Masafumi

    2014-01-01

    For the development and optimization of materials processing a collection of thermodynamic information concerning substances that participate in the reactions is important. One fundamental way to obtain such information is to measure the vapor pressure of gas species under conditions where they are in equilibrium with the condensed phases. Over the past 60 years Knudsen cell mass spectrometry has been used to identify and quantitatively determine gas species at high temperatures. This article describes thermodynamic foundation and examples of measurements in order to demonstrate the use of mass spectrometry focusing on the field of process metallurgy and recycling processes. PMID:26819884

  6. Measurement of gamma-ray production cross sections in neutron-induced reactions for Al and Pb

    SciTech Connect

    Pavlik, A.; Vonach, H.; Hitzenberger, H.; Nelson, R.O.; Haight, R.C.; Wender, S.A.; Young, P.G.; Chadwick, M.B.

    1995-02-01

    The prompt gamma-radiation from the interaction of fast neutrons with aluminum and lead was measured using the white neutron beam of the WNR facility at the Los Alamos National Laboratory. The samples (Al and isotopically enriched {sup 207}Pb and {sup 208}Pb) were positioned at about 20 m or 41 m distance from the neutron production target. The spectra of the emitted gamma-rays were measured with a high-resolution HPGe detector. The incident neutron energy was determined by the time-of-flight method and the neutron fluence was measured with a U fission chamber. From the aluminum gamma-ray spectra excitation functions for prominent gamma-transitions in various residual nuclei (in the range from O to Al) were derived for neutron energies from 3 MeV to 400 MeV. For lead (n,xn{gamma}) reactions were studied for neutron energies up to 200 MeV by analyzing prominent gamma-transitions in the residual nuclei {sup 200,202,204,206,207,208}Pb. The experimental results were compared with nuclear model calculations using the code GNASH. A good overall agreement was obtained without special parameter adjustments.

  7. Finite Larmor radii effects in fast ion measurements with neutron emission spectrometry

    NASA Astrophysics Data System (ADS)

    Eriksson, J.; Hellesen, C.; Andersson Sundén, E.; Cecconello, M.; Conroy, S.; Ericsson, G.; Gatu Johnson, M.; Pinches, S. D.; Sharapov, S. E.; Weiszflog, M.; EFDA contributors, JET

    2013-01-01

    When analysing data from fast ion measurements it is normally assumed that the gyro-phase distribution of the ions is isotropic within the field of view of the measuring instrument. This assumption is not valid if the Larmor radii of the fast ions are comparable to—or larger than—the gradient scale length in the spatial distribution of the ions, and if this scale length is comparable to—or smaller than—the width of the field of view of the measuring instrument. In this paper the effect of such an anisotropy is demonstrated by analysing neutron emission spectrometry data from a JET experiment with deuterium neutral beams together with radiofrequency heating at the third harmonic of the deuterium cyclotron frequency. In the experiment, the neutron time-of-flight spectrometer TOFOR was used to measure the neutrons from the d(d,n)3He-reaction. Comparison of the experimental data with Monte Carlo calculations shows that the finite Larmor radii of the fast ions need to be included in the modelling to get a good description of the data. Similar effects are likely to be important for other fast ion diagnostics, such as γ-ray spectroscopy and neutral particle analysis, as well.

  8. Protein turnover measurement using selected reaction monitoring-mass spectrometry (SRM-MS).

    PubMed

    Holman, Stephen W; Hammond, Dean E; Simpson, Deborah M; Waters, John; Hurst, Jane L; Beynon, Robert J

    2016-10-28

    Protein turnover represents an important mechanism in the functioning of cells, with deregulated synthesis and degradation of proteins implicated in many diseased states. Therefore, proteomics strategies to measure turnover rates with high confidence are of vital importance to understanding many biological processes. In this study, the more widely used approach of non-targeted precursor ion signal intensity (MS1) quantification is compared with selected reaction monitoring (SRM), a data acquisition strategy that records data for specific peptides, to determine if improved quantitative data would be obtained using a targeted quantification approach. Using mouse liver as a model system, turnover measurement of four tricarboxylic acid cycle proteins was performed using both MS1 and SRM quantification strategies. SRM outperformed MS1 in terms of sensitivity and selectivity of measurement, allowing more confident determination of protein turnover rates. SRM data are acquired using cheaper and more widely available tandem quadrupole mass spectrometers, making the approach accessible to a larger number of researchers than MS1 quantification, which is best performed on high mass resolution instruments. SRM acquisition is ideally suited to focused studies where the turnover of tens of proteins is measured, making it applicable in determining the dynamics of proteins complexes and complete metabolic pathways.This article is part of the themed issue 'Quantitative mass spectrometry'. PMID:27644981

  9. Plutonium gamma-ray measurements for mutual reciprocal inspections of dismantled nuclear weapons

    SciTech Connect

    Koenig, Z.M.; Carlson, J.B.; Clark, D.; Gosnell, T.B.

    1995-07-01

    The O`Leary-Mikhailov agreement of March 1994 stated that the U.S. and the Russian Federation would engage in mutual reciprocal inspections (MRI) of fissile materials removed from dismantled nuclear weapons. It was decided to begin with the plutonium (Pu) removed from dismantled weapons and held in storage containers. Later discussions between U.S. and Russian technical experts led to the conclusion that, to achieve the O`Leary-Mikhailov objectives, Pu MRI would need to determine that the material in the containers has properties consistent with a nuclear-weapon component. Such a property is a {sup 240}Pu/{sup 239}Pu ratio consistent with weapons-grade material. One of the candidate inspection techniques under consideration for Pu MRI is to use a narrow region (630-670 keV) of the plutonium gamma-ray spectrum, taken with a high-purity germanium detector, to determine that it is weapons-grade plutonium as well as to estimate the minimum mass necessary to produce the observed gamma-ray intensity. We developed software (the Pu600 code) for instrument control and analysis especially for this purpose. In November 1994, U.S. and Russian scientists met at the Lawrence Livermore National Laboratory for joint experiments to evaluate candidate Pu MRI inspection techniques. In one of these experiments, gamma-ray intensities were measured from three unclassified weapons-grade plutonium source standards and one reactor-grade standard (21% {sup 240}pu). Using our software, we determined the {sup 240}Pu/{sup 239}Pu ratio of these standards to accuracies within {+-}10%, which is adequate for Pu MRI. The minimum mass estimates varied, as expected, directly with the exposed surface area of the standards.

  10. Measurement of direct photon emission in the K(L) ---> pi+ pi- gamma decay mode

    SciTech Connect

    Abouzaid, E.; Arenton, M.; Barker, A.R.; Bellantoni, L.; Bellavance, A.; Blucher, E.; Bock, G.J.; Cheu, E.; Coleman, R.; Corcoran, M.D.; Corti, G.; /Virginia U. /Wisconsin U., Madison

    2006-04-01

    In this paper the KTeV collaboration reports the analysis of 112.1 x 10{sup 3} candidate K{sub L} {yields} {pi}{sup +}{pi}{sup -}{gamma} decays including a background of 671 {+-} 41 events with the objective of determining the photon production mechanisms intrinsic to the decay process. These decays have been analyzed to extract the relative contributions of the Cp violating bremsstrahlung process and the CP conserving M1 and CP violating E1 direct photon emission processes. The M1 direct photon emission amplitude and its associated vector form factor parameterized as |{bar g}{sub M1}|(1 + a{sub 1}/a{sub 2}/(M{sub {rho}}{sup 2}-M{sub K}{sup 2}) + 2M{sub K}E{sub {gamma}}) have been measured to be |{bar g}{sub M1}| = 1.198 {+-} 0.035(stat) {+-} 0.086(syst) and a{sub 1}/a{sub 2} = =0.738 {+-} 0.007(stat) {+-} 0.018(syst) GeV{sup 2}/c{sup 2} respectively. An upper limit for the CP violating E1 direct emission amplitude |g{sub E1}| {le} 0.1 (90%CL) has been found. The overall ratio of direct photon emission (DE) to total photon emission including the bremsstrahlung process (IB) has been determined to be DE/(DE + IB) = 0.689 {+-} 0.021 for E{sub {gamma}} {ge} 20 MeV.

  11. Accelerator Mass Spectrometry Measurements of Plutonium in Sediment and Seawater from the Marshall Islands

    SciTech Connect

    Leisvik, M; Hamilton, T

    2001-08-01

    During the summer 2000, I was given the opportunity to work for about three months as a technical trainee at Lawrence Livermore National Laboratory, or LLNL as I will refer to it hereafter. University of California runs this Department of Energy laboratory, which is located 70 km east of San Francisco, in the small city of Livermore. This master thesis in Radioecology is based on the work I did here. LLNL, as a second U.S.-facility for development of nuclear weapons, was built in Livermore in the beginning of the 1950's (Los Alamos in New Mexico was the other one). It has since then also become a 'science center' for a number of areas like magnetic and laser fusion energy, non-nuclear energy, biomedicine, and environmental science. The Laboratory's mission has changed over the years to meet new national needs. The following two statements were found on the homepage of LLNL (http://www.llnl.gov), at 2001-03-05, where also information about the laboratory and the scientific projects that takes place there, can be found. 'Our primary mission is to ensure that the nation's nuclear weapons remain safe, secure, and reliable and to prevent the spread and use of nuclear weapons worldwide'. 'Our goal is to apply the best science and technology to enhance the security and well-being of the nation and to make the world a safer place.' The Marshall Islands Dose Assessment and Radioecology group at the Health and Ecological Assessments division employed me, and I also worked to some extent with the Centre for Accelerator Mass Spectrometry (CAMS) group. The work I did at LLNL can be divided into two parts. In the first part Plutonium (Pu) measurements in sediments from the Rongelap atoll in Marshall Islands, using Accelerator Mass Spectrometry (AMS) were done. The method for measuring these kinds of samples is well understood at LLNL since soil samples have been measured with AMS for Pu in the past. Therefore it was the results that were of main interest and not the technique

  12. High performance gamma measurements of equipment retrieved from Hanford high-level nuclear waste tanks

    SciTech Connect

    Troyer, G.L.

    1997-03-17

    The cleanup of high level defense nuclear waste at the Hanford site presents several progressive challenges. Among these is the removal and disposal of various components from buried active waste tanks to allow new equipment insertion or hazards mitigation. A unique automated retrieval system at the tank provides for retrieval, high pressure washing, inventory measurement, and containment for disposal. Key to the inventory measurement is a three detector HPGe high performance gamma spectroscopy system capable of recovering data at up to 90% saturation (200,000 counts per second). Data recovery is based on a unique embedded electronic pulser and specialized software to report the inventory. Each of the detectors have different shielding specified through Monte Carlo simulation with the MCNP program. This shielding provides performance over a dynamic range of eight orders of magnitude. System description, calibration issues and operational experiences are discussed.

  13. Spectroscopic measurement of impurity ion behavior in the GAMMA10 tandem mirror

    NASA Astrophysics Data System (ADS)

    Ikeda, K.; Nagayama, Y.; Itoh, T.; Kawamori, E.; Okamoto, Y.; Tamano, T.; Yamaguchi, N.; Yatsu, K.; Yoshikawa, M.

    1999-01-01

    Behavior of impurity ions has been investigated using visible spectroscopy in the GAMMA10 tandem mirror. A 40 channel visible spectrometer system has been developed for measurements of the ion temperature and ion flow velocity. The spectrometer consists of a 100 cm monochromator, a 40 channel optical fiber array and an image intensifier tube coupled with a charge coupled device TV camera. The spectra from low ionization states of oxygen and carbon are measured in ion cyclotron range of frequency heated plasmas. High ion temperatures (3-10 keV) of O4+ are observed in the anchor region, where the minimum B mirror field is produced by baseball coils. The O4+ ion is heated by the fourth harmonic frequency of O4+, which is most likely due to the cyclotron higher harmonic damping.

  14. Measuring Ω_M and Ω_Λ with long-duration gamma-ray bursts

    NASA Astrophysics Data System (ADS)

    Balastegui, A.; Canal, R.; Ruiz-Lapuente, P.

    2010-08-01

    Gamma-ray bursts (GRBs) are one of the most luminous events in the Universe. In addition, the Universe itself is almost transparent to γ-rays, making GRBs detectable up to very high redshifts. As a result, GRBs are very suitable to probe the cosmological parameters. This work shows the potential of long-duration GRBs for measuring the cosmological parameters Ω_M and Ω_Λ by comparing the observed log N-log P distribution with the theoretical one. Provided that the GRBs rate and luminosity function are well determined, the best values and 1σ confidence intervals obtained are Ω_M=0.22+0.05-0.03 and Ω_Λ=1.06+0.05-0.10. Finally, a set of simulations show the ability of the method to measure Ω_M and Ω_Λ.

  15. Glucose and glycerol concentrations and their tracer enrichment measurements using liquid chromatography tandem mass spectrometry.

    PubMed

    Bornø, Andreas; Foged, Lene; van Hall, Gerrit

    2014-10-01

    The present study describes a new liquid chromatography tandem mass spectrometry method for high-throughput quantification of glucose and glycerol in human plasma using stable isotopically labeled internal standards and is suitable for simultaneous measurements of glucose and glycerol enrichments in connection to in vivo metabolic studies investigating glucose turnover and lipolytic rate. Moreover, in order to keep up with this new fast analysis, simple derivatization procedures have been developed. Prior to analysis, glucose and glycerol were derivatized using benzoyl chloride in order to form benzoylated derivatives via new simplified fast procedures. For glucose, two internal standards were evaluated, [U-(13) C(6)]glucose and [U-(13) C(6), D(7)]glucose, and for glycerol, [U-(13) C(3), D(8)]glycerol was used. The method was validated by means of calibration curves, quality control samples, and plasma samples spiked with [6,6-D(2)]glucose, [U-(13) C(6)]glucose, and [1,1,2,3,3-D(5)]glycerol in order to test accuracy, precision, and recovery of the method. Moreover, post preparative and freeze-thaw sample stability were tested. The correlation of calibration curves for the glucose concentration were r(2) = 0.9998 for [U-(13) C(6)]glucose and r(2) = 0.9996 for [U-(13) C(6), D(7)]glucose, and r(2) = 0.9995 for the glycerol concentration. Interday accuracy for glucose using [U-(13) C(6)]glucose and glycerol determined in spiked plasma were respectively 103.5% and 106.0%, and the coefficients of variation were 2.0% and 9.7%, respectively. After derivatization, plasma samples were stable for at least 14 days. In conclusion, we have developed and validated a novel, accurate, and sensitive high-throughput liquid chromatography tandem mass spectrometry method for simultaneous determination of glucose and glycerol concentrations and enrichment of infused tracers most commonly used in human metabolic kinetic studies.

  16. An improved method for measuring metaldehyde in surface water using liquid chromatography tandem mass spectrometry

    PubMed Central

    Schumacher, Melanie; Castle, Glenn; Gravell, Anthony; Mills, Graham A.; Fones, Gary R.

    2016-01-01

    The molluscicide metaldehyde (2,4,6,8-tetramethyl-1,3,5,7-tetraoxocanemetacetaldehyde) is an emerging pollutant. It is frequently detected in surface waters, often above the European Community Drinking Water Directive limit of 0.1 μg/L for a single pesticide. Gas chromatography mass spectrometry (GC–MS) can be used to determine metaldehyde in environmental waters, but this method requires time consuming extraction techniques prior to instrumental analysis. Use of liquid chromatography-tandem mass spectrometry (LC–MS/MS) can overcome this problem. We describe a novel LC–MS/MS method, using a methylamine mobile phase additive, coupled with on-line sample enrichment that allows for the rapid and sensitive measurement of metaldehyde in surface water. Only the methylamine adduct of metaldehyde was formed with other unwanted alkali metal adducts and dimers being suppressed. As considerably less collision energy is required to fragment the methylamine adduct, a five-fold improvement in method sensitivity, compared to a previous method using an ammonium acetate buffer mobile phase was achieved. This new approach offers: • A validated method that meets regulatory requirements for the determination of metaldehyde in surface water. • Improved reliability of quantification over existing LC–MS/MS methods by using stable precursor ions for multiple reaction monitoring. • Low limits of quantification for tap water (4 ng/L) and river water (20 ng/L) using only 800 μL of sample; recoveries > 97%. PMID:27054094

  17. Comparison of FTIR and Particle Mass Spectrometry for the Measurement of Paticulate Organic Nitrates

    SciTech Connect

    Bruns, Emily; Perraud, Veronique; Zelenyuk, Alla; Ezell, Michael J.; Johnson, Stanley N.; Yu, Yong; Imre, D.; Finlayson-Pitts, Barbara J.; Alexander, M. L.

    2010-02-01

    While multifunctional organic nitrates are formed during the atmospheric oxidation of volatile organic compounds, relatively little is known about their signatures in particle mass spectrometers. High resolution time-of-flight aerosol mass spectrometry (HR-ToF-AMS) was applied to NH4NO3, NaNO3 and isosorbide 5-mononitrate (IMN) particles, and to secondary organic aerosol (SOA) from NO3 radical reactions at 22 C and 1 atm in air with and pinene, 3-carene, limonene and isoprene. For comparison, single particle laser ablation mass spectra (SPLAT II) were also obtained for IMN and SOA from the pinene reaction. The mass spectra of all particles exhibit significant intensity at m/z 30, and for the SOA, weak peaks corresponding to various organic fragments containing nitrogen [CxHyNzOa]+ were identified using HR-ToF-AMS. The NO+/NO2+ ratios from HR-ToF-AMS were 10-15 for IMN and the SOA from the and pinene, 3-carene and limonene reactions, ~5 for the isoprene reaction, 2.4 for NH4NO3 and 80 for NaNO3. The N/H ratios from HR-ToF-AMS for the SOA were smaller by a factor of 2 to 4 than the -ONO2/C-H ratios measured using FTIR on particles impacted on ZnSe windows. While the NO+/NO2+ ratio may provide a generic indication of organic nitrates under some conditions, specific identification of particulate organic nitrates awaits further development of particle mass spectrometry techniques.

  18. Quantitative measurements of small molecule mixtures using laser electrospray mass spectrometry.

    PubMed

    Flanigan, Paul M; Perez, Johnny J; Karki, Santosh; Levis, Robert J

    2013-04-01

    Quantitative measurements of atenolol, tioconazole, tetraethylammonium bromide, and tetrabutylammonium iodide using laser electrospray mass spectrometry (LEMS) reveal monotonic signal response as a function of concentration for single analytes, two- and four-component equimolar mixtures, and two-component variable molarity mixtures. LEMS analyses of single analytes as a function of concentration were linear over ~2.5 orders of magnitude for all four analytes and displayed no sign of saturation. Corresponding electrospray ionization (ESI) measurements displayed a nonmonotonic increase as saturation occurred at higher concentrations. In contrast to the LEMS experiments, the intensity ratios from control experiments using conventional ESI-MS deviated from expected values for the equimolar mixture measurements due to ion suppression of less surface active analytes, particularly in the analysis of the four-component mixture. In the analyses of two-component nonequimolar mixtures, both techniques were able to determine the concentration ratios after adjustment with response factors although conventional ESI-MS was subject to a greater degree of saturation and ion suppression at higher analyte concentrations.

  19. Remote measurement of highly toxic vapors by scanning imaging Fourier-transform spectrometry

    NASA Astrophysics Data System (ADS)

    Harig, Roland; Rusch, Peter; Dyer, Chris; Jones, Anita; Moseley, Richard; Truscott, Benjamin

    2005-11-01

    In the case of chemical accidents, terrorist attacks, or war, hazardous compounds may be released into the atmosphere. Remote sensing by Fourier-transform infrared spectrometry allows identification and quantification of these hazardous clouds. The output of current standoff detection systems is a yes/no decision by an automatic identification algorithm that analyses the measured spectrum. The interpretation of the measured spectrum by the operator is complicated and thus this task requires an expert. Even if a scanning system is used for surveillance of a large area the operator is dependent on the decision of the algorithm. In contrast to that, imaging systems allow automatic identification but also simple interpretation of the result, the image of the cloud. Therefore, an imaging spectrometer, the scanning infrared gas imaging system (SIGIS) has been developed. The system is based on an interferometer with a single detector element (Bruker OPAG 22) in combination with a telescope and a synchronised scanning mirror. The results of the analyses of the spectra are displayed by an overlay of a false colour image, the "chemical cloud image", on a video image. In this work, the first application of the system as chemical warfare agent identification and imaging system is described. The system, the data analysis method, and results of measurements of chemical warfare agents are presented.

  20. Acid effects on the measurement of mercury by cold vapor atomic absorption spectrometry

    SciTech Connect

    Adeloju, S.B.; Mann, T.F.

    1987-07-01

    The influence of nitric, hydrochloric and sulfuric acids on the measurement of mercury by cold vapor atomic absorption spectrometry has been investigated. Small pre-reduction peaks associated with the instability of mercury were observed in solutions containing less than or equal to 12.5, < 2 and less than or equal to 12.5% v/v of each acid, respectively. Mercury was found to be most stable in greater than or equal to 2% v/v hydrochloric acid and the measured absorbance was not greatly influenced by varying concentration of the acid. The mercury absorbance measurements were more sensitive in solutions containing less than or equal to 6.3% v/v hydrochloric acid than in similar concentrations of nitric and sulfuric acids. The use of the three acids as a digestion mixture result in serious interference from nitrogen oxides. The interference was removed by use of expelling agents such as urea and sulfamic acid or overcome by use of excess stannous chloride, prior to the reduction of mercury(II) ions. The determination of mercury in NBS albacore tuna using both of these approaches to overcome the interference problem proved to be successful.

  1. Measurement of Inclusive Radiative B -Meson Decay B -> X_s gamma

    SciTech Connect

    Ozcan, V.E.; /SLAC /Stanford U., Appl. Phys. Dept.

    2006-01-06

    Radiative decays of the B meson, B {yields} X{sub s}{gamma}, proceed via virtual flavor changing neutral current processes that are sensitive to contributions from high mass scales, either within the Standard Model of electroweak interactions or beyond. In the Standard Model, these transitions are sensitive to the weak interactions of the top quark, and relatively robust predictions of the inclusive decay rate exist. Significant deviation from these predictions could be interpreted as indications for processes not included in the minimal Standard Model, like interactions of charged Higgs or SUSY particles. The analysis of the inclusive photon spectrum from B {yields} X{sub s}{gamma} decays is rather challenging due to high backgrounds from photons emitted in the decay of mesons in B decays as well as e{sup +}e{sup -} annihilation to low mass quark and lepton pairs. Based on 88.5 million B{bar B} events collected by the BABAR detector, the photon spectrum above 1.9 GeV is presented. By comparison of the first and second moments of the photon spectrum with QCD predictions (calculated in the kinetic scheme), QCD parameters describing the bound state of the b quark in the B meson are extracted: m{sub b} = (4.45 {+-} 0.16) GeV/c{sup 2}; {mu}{sub {pi}}{sup 2} = (0.65 {+-} 0.29) GeV{sup 2}. These parameters are useful input to non-perturbative QCD corrections to the semileptonic B decay rate and the determination of the CKM parameter |V{sub ub}|. Based on these parameters and heavy quark expansion, the full branching fraction is obtained as: {Beta}(B {yields} X{sub s}{gamma}){sup E{sub {gamma}}>1.6 GeV} = (4.05 {+-} 0.32(stat) {+-} 0.38(syst) {+-} 0.29(model)) x 10{sup -4}. This result is in good agreement with previous measurements, the statistical and systematic errors are comparable. It is also in good agreement with the theoretical Standard Model predictions, and thus within the present errors there is no indication of any interactions not accounted for in the

  2. REAL-TIME IN-SITU MEASUREMENT OF MATERIAL ELASTIC PROPERTIES IN A HIGH GAMMA IRRADIATION ENVIRONMENT

    SciTech Connect

    Ken Telschow; Rob Schley; Dave Cottle

    2006-05-01

    The first measurements of elastic vibrations of an object in-situ to a high gamma irradiation field using a laser coupled resonant ultrasound method are described. A vibration mode of an Inconel hollow capped cylinder was measured throughout a period of 170 hours as the gamma radiation field was increased to 104 Gray/hour. The vibration mode frequency was observed to change in a manner consistent with the temperature dependence of the elastic stiffness coefficients of the material. These results illustrate the efficacy of the laser approach for real-time resonant ultrasound measurements in this severely hostile nuclear environment.

  3. Single-source gamma radiation procedures for improved calibration and measurements in porous media

    SciTech Connect

    Oostrom, M.; Hofstee, C.; Dane, H.; Lenhard, R.J.

    1998-08-01

    When dual-energy gamma radiation systems are employed for measurements in porous media, count rates from both sources are often used to compute parameter values. However, for several applications, the count rates of just one source are insufficient. These applications include the determination of volumetric liquid content values in two-liquid systems and salt concentration values in water-saturated porous media. Single-energy gamma radiation procedures for three applications are described in this paper. Through an error analysis, single-source procedures are shown to reduce the probable error in the determinations considerably. Example calculations and simple column experiments were conducted for each application to compare the performance of the new single-source and standard dual-source methods. In all cases, the single-source methods provided more reliable data than the traditional dual-source methods. In addition, a single-source calibration procedure is proposed to determine incident count rates indirectly. This procedure, which requires packing under saturated conditions, can be used in all single- and dual-source applications and yields accurate porosity and dry bulk density values.

  4. Measurements of the reaction e/+/e/-/ yielding gamma-gamma at center-of-mass energies in the range 6.2-7.4 GeV

    NASA Technical Reports Server (NTRS)

    Hilger, E.; Beron, B. L.; Carrington, R. L.; Ford, R. L.; Hill, W. T.; Hofstadter, R.; Hughes, E. B.; Liberman, A. D.; Martin, T. W.; Oneill, L. H.

    1977-01-01

    The cross section for the pair-annihilation reaction e(+)e(-) yields gamma-gamma were measured at center-of-mass energies in the range 6.2-7.4 GeV and at production angles close to 90 deg. The experimental apparatus consisted of two identical spectrometers which were set to view the luminous region at SPEAR-II from opposite directions at an azimuthal angle of 45 deg. In each spectrometer there was a NaI(TI) crystal 20 radiation lengths thick and 30 in. in diameter to measure the gamma-ray energies. Annihilation events were detected by an electronic trigger which required only the observation in coincidence of more than 0.2 GeV in each NaI(TI) crystal within + or - 15 nsec of the crossing beams. The observed rates of pair-annihilation events were found to be in agreement with those expected from quantum electrodynamics (QED) at all the center-of-mass energies used.

  5. Arcsec source location measurements in gamma-ray astronomy from a lunar observatory

    NASA Technical Reports Server (NTRS)

    Koch, David G.; Hughes, E. B.

    1990-01-01

    The physical processes typically used in the detection of high energy gamma-rays do not permit good angular resolution, which makes difficult the unambiguous association of discrete gamma-ray sources with objects emitting at other wavelengths. This problem can be overcome by placing gamma-ray detectors on the moon and using the horizon as an occulting edge to achieve arcsec resolution. For the purpose of discussion, this concept is examined for gamma rays above about 20 MeV for which pair production dominates the detection process and locally-generated nuclear gamma rays do not contribute to the background.

  6. Measurement of the 21Na(p,{gamma})22Mg Reaction with the Dragon Facility at TRIUMF-ISAC

    SciTech Connect

    Chen, A.A.; Bishop, S.; D'Auria, J.M.; Hunter, D.; Lamey, M.; Liu, W.; Wrede, C.; Buchmann, L.; Hutcheon, D.A.; Laird, A.; Ottewell, D.; Rogers, J.; Chatterjee, M. L.; Engel, S.; Strieder, F.; Gigliotti, D.; Hussein, A.; Greife, U.; Jewett, C.; King, J.

    2003-08-26

    The DRAGON recoil separator facility, designed to measure the rates of radiative proton and alpha capture reactions important for nuclear astrophysics, is now operational at the TRIUMF-ISAC radioactive beam facility in Vancouver, Canada. We report on first measurements of the 21Na(p,{gamma})22Mg reaction rate with radioactive beams of 21Na.

  7. Operation GREENHOUSE. Scientific Director's report. Annex 1. 1. Prompt-gamma-ray measurements. Part 4. Installation drawings. Nuclear explosions 1951

    SciTech Connect

    Hall, W.C.

    1984-10-31

    This report consists of drawings and tabular data pertinent to the various measurements performed in Operation GREENHOUSE. The drawings represent the plans for the cable installations, recorder stations, power and signal lines, and other equipment used in the measurement of prompt gamma rays, alpha, transit time, neutron intensity (Tenex), and thermal radiation.

  8. Direct Measurement of Free Estradiol in Human Serum and Plasma by Equilibrium Dialysis-Liquid Chromatography-Tandem Mass Spectrometry.

    PubMed

    Ray, Julie A; Kushnir, Mark M; Rockwood, Alan L; Meikle, A Wayne

    2016-01-01

    We describe a direct method of measurement of free estradiol using equilibrium dialysis followed by liquid chromatography-tandem mass spectrometry (LC-MS/MS). Serum aliquots and internal standards are extracted by liquid-liquid extraction using methyl-tert-butyl ether (MTBE) followed by derivatization with dansyl chloride. An API 5500 mass spectrometer operated in positive electrospray mode is used for detection.

  9. Polyethylene-reflected plutonium metal sphere : subcritical neutron and gamma measurements.

    SciTech Connect

    Mattingly, John K.

    2009-11-01

    Numerous benchmark measurements have been performed to enable developers of neutron transport models and codes to evaluate the accuracy of their calculations. In particular, for criticality safety applications, the International Criticality Safety Benchmark Experiment Program (ICSBEP) annually publishes a handbook of critical and subcritical benchmarks. Relatively fewer benchmark measurements have been performed to validate photon transport models and codes, and unlike the ICSBEP, there is no program dedicated to the evaluation and publication of photon benchmarks. Even fewer coupled neutron-photon benchmarks have been performed. This report documents a coupled neutron-photon benchmark for plutonium metal reflected by polyethylene. A 4.5-kg sphere of ?-phase, weapons-grade plutonium metal was measured in six reflected configurations: (1) Bare; (2) Reflected by 0.5 inch of high density polyethylene (HDPE); (3) Reflected by 1.0 inch of HDPE; (4) Reflected by 1.5 inches of HDPE; (5) Reflected by 3.0 inches of HDPE; and (6) Reflected by 6.0 inches of HDPE. Neutron and photon emissions from the plutonium sphere were measured using three instruments: (1) A gross neutron counter; (2) A neutron multiplicity counter; and (3) A high-resolution gamma spectrometer. This report documents the experimental conditions and results in detail sufficient to permit developers of radiation transport models and codes to construct models of the experiments and to compare their calculations to the measurements. All of the data acquired during this series of experiments are available upon request.

  10. Dissolved atmospheric gas in xylem sap measured with membrane inlet mass spectrometry.

    PubMed

    Schenk, H Jochen; Espino, Susana; Visser, Ate; Esser, Bradley K

    2016-04-01

    A new method is described for measuring dissolved gas concentrations in small volumes of xylem sap using membrane inlet mass spectrometry. The technique can be used to determine concentrations of atmospheric gases, such as argon, as reported here, or for any dissolved gases and their isotopes for a variety of applications, such as rapid detection of trace gases from groundwater only hours after they were taken up by trees and rooting depth estimation. Atmospheric gas content in xylem sap directly affects the conditions and mechanisms that allow for gas removal from xylem embolisms, because gas can dissolve into saturated or supersaturated sap only under gas pressure that is above atmospheric pressure. The method was tested for red trumpet vine, Distictis buccinatoria (Bignoniaceae), by measuring atmospheric gas concentrations in sap collected at times of minimum and maximum daily temperature and during temperature increase and decline. Mean argon concentration in xylem sap did not differ significantly from saturation levels for the temperature and pressure conditions at any time of collection, but more than 40% of all samples were supersaturated, especially during the warm parts of day. There was no significant diurnal pattern, due to high variability between samples.

  11. On copper diffusion in silicon measured by glow discharge mass spectrometry.

    PubMed

    Modanese, Chiara; Gaspar, Guilherme; Arnberg, Lars; Di Sabatino, Marisa

    2014-11-01

    Copper contamination occurs frequently in silicon for photovoltaic applications due to its very fast diffusion coupled with a low solid solubility, especially at room temperature. The combination of these properties exerts a challenge on the direct analysis of Cu bulk concentration in Si by sputtering techniques like glow discharge mass spectrometry (GDMS). This work aims at addressing the challenges in quantitative analysis of fast diffusing elements in Si matrix by GDMS. N-type, monocrystalline (Czochralski) silicon samples were intentionally contaminated with Cu after solidification and consequently annealed at 900 °C to ensure a homogeneous distribution of Cu in the bulk. The samples were quenched after annealing to control the extent of the diffusion to the surface prior to the GDMS analyses, which were carried out at different time intervals from within few minutes after cooling onward. The Cu profiles were measured by high-resolution GDMS operating in a continuous direct current mode, where the integration step length was set to ∼0.5 μm over a total sputtered depth of 8-30 μm. The temperature of the samples during the GDMS analyses was also measured in order to evaluate the diffusion. The Cu contamination of n-type Si samples was observed to be highly material dependent. The practical impact of Cu out-diffusion on the calculation of the relative sensitivity factor (RSF) of Cu in Si is discussed.

  12. Dissolved atmospheric gas in xylem sap measured with membrane inlet mass spectrometry.

    PubMed

    Schenk, H Jochen; Espino, Susana; Visser, Ate; Esser, Bradley K

    2016-04-01

    A new method is described for measuring dissolved gas concentrations in small volumes of xylem sap using membrane inlet mass spectrometry. The technique can be used to determine concentrations of atmospheric gases, such as argon, as reported here, or for any dissolved gases and their isotopes for a variety of applications, such as rapid detection of trace gases from groundwater only hours after they were taken up by trees and rooting depth estimation. Atmospheric gas content in xylem sap directly affects the conditions and mechanisms that allow for gas removal from xylem embolisms, because gas can dissolve into saturated or supersaturated sap only under gas pressure that is above atmospheric pressure. The method was tested for red trumpet vine, Distictis buccinatoria (Bignoniaceae), by measuring atmospheric gas concentrations in sap collected at times of minimum and maximum daily temperature and during temperature increase and decline. Mean argon concentration in xylem sap did not differ significantly from saturation levels for the temperature and pressure conditions at any time of collection, but more than 40% of all samples were supersaturated, especially during the warm parts of day. There was no significant diurnal pattern, due to high variability between samples. PMID:26868162

  13. Real-time measurement of sodium chloride in individual aerosol particles by mass spectrometry

    NASA Technical Reports Server (NTRS)

    Sinha, M. P.; Friedlander, S. K.

    1985-01-01

    The method of particle analysis by mass spectrometry has been applied to the quantitative measurement of sodium chloride in individual particles on a real-time basis. Particles of known masses are individually introduced, in the form of a beam, into a miniature Knudsen cell oven (1600 K). The oven is fabricated from rhenium metal sheet (0.018 mm thick) and is situated in the ion source of a quadrupole mass spectrometer. A particle once inside the oven is trapped and completely volatilized; this overcomes the problem of partial volatilization due to particles bouncing from the filament surface. Individual particles are thermally volatilized and ionized inside the rhenium oven, and produce discrete sodium ion pulses whose intensities are measured with the quadrupole mass spectrometer. An ion pulse width of several milliseconds (4-12 ms) is found for particles in the mass range 1.3 x 10 to the -13th to 5.4 x 10 to the -11th g. The sodium ion intensity is found to be proportional to the particle mass to the 0.86-power. The intensity distribution for monodisperse aerosol particles possesses a geometric standard deviation of 1.09, showing that the method can be used for the determination of the mass distribution function with good resolution in a polydisperse aerosol.

  14. Determining the radon exhalation rate from a gold mine tailings dump by measuring the gamma radiation.

    PubMed

    Ongori, Joash N; Lindsay, Robert; Newman, Richard T; Maleka, Peane P

    2015-02-01

    The mining activities taking place in Gauteng province, South Africa have caused millions of tons of rocks to be taken from underground to be milled and processed to extract gold. The uranium bearing tailings are placed in an estimated 250 dumps covering a total area of about 7000 ha. These tailings dumps contain considerable amounts of radium and have therefore been identified as large sources of radon. The size of these dumps make traditional radon exhalation measurements time consuming and it is difficult to get representative measurements for the whole dump. In this work radon exhalation measurements from the non-operational Kloof mine dump have been performed by measuring the gamma radiation from the dump fairly accurately over an area of more than 1 km(2). Radon exhalation from the mine dump have been inferred from this by laboratory-based and in-situ gamma measurements. Thirty four soil samples were collected at depths of 30 cm and 50 cm. The weighted average activity concentrations in the soil samples were 308 ± 7 Bq kg(-1), 255 ± 5 Bq kg(-1) and 18 ± 1 Bq kg(-1) for (238)U, (40)K and (232)Th, respectively. The MEDUSA (Multi-Element Detector for Underwater Sediment Activity) γ-ray detection system was used for field measurements. The radium concentrations were then used with soil parameters to obtain the radon flux using different approaches such as the IAEA (International Atomic Energy Agency) formula. Another technique the MEDUSA Laboratory Technique (MELT) was developed to map radon exhalation based on (1) recognising that radon exhalation does not affect (40)K and (232)Th activity concentrations and (2) that the ratio of the activity concentration of the field (MEDUSA) to the laboratory (HPGe) for (238)U and (40)K or (238)U and (232)Th will give a measure of the radon exhalation at a particular location in the dump. The average, normalised radon flux was found to be 0.12 ± 0.02 Bq m(-2) s(-1) for the mine dump. PMID:25461511

  15. Determining the radon exhalation rate from a gold mine tailings dump by measuring the gamma radiation.