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Sample records for high-gain harmonic generation

  1. High gain amplifiers: Power oscillations and harmonic generation

    SciTech Connect

    Dattoli, G.; Ottaviani, P. L.; Pagnutti, S.

    2007-08-01

    We discuss the power oscillations in saturated high gain free electron laser amplifiers and show that the relevant period can be written in terms of the gain length. We use simple arguments following from the solution of the pendulum equation in terms of Jacobi elliptic functions. Nontrivial effects due to nonlinear harmonic generation and inhomogeneous broadening are discussed too, as well as the saturated dynamics of short pulses.

  2. STARS A Two Stage High Gain Harmonic Generation FEL Demonstrator

    SciTech Connect

    M. Abo-Bakr; W. Anders; J. Bahrdt; P. Budz; K.B. Buerkmann-Gehrlein; O. Dressler; H.A. Duerr; V. Duerr; W. Eberhardt; S. Eisebitt; J. Feikes; R. Follath; A. Gaupp; R. Goergen; K. Goldammer; S.C. Hessler; K. Holldack; E. Jaeschke; Thorsten Kamps; S. Klauke; J. Knobloch; O. Kugeler; B.C. Kuske; P. Kuske; A. Meseck; R. Mitzner; R. Mueller; M. Neeb; A. Neumann; K. Ott; D. Pfluckhahn; T. Quast; M. Scheer; Th. Schroeter; M. Schuster; F. Senf; G. Wuestefeld; D. Kramer; Frank Marhauser

    2007-08-01

    BESSY is proposing a demonstration facility, called STARS, for a two-stage high-gain harmonic generation free electron laser (HGHG FEL). STARS is planned for lasing in the wavelength range 40 to 70 nm, requiring a beam energy of 325 MeV. The facility consists of a normal conducting gun, three superconducting TESLA-type acceleration modules modified for CW operation, a single stage bunch compressor and finally a two-stage HGHG cascaded FEL. This paper describes the faciliy layout and the rationale behind the operation parameters.

  3. Nonlinear harmonic generation in high-gain free-electron lasers

    SciTech Connect

    Dattoli, G.; Ottaviani, P.L.; Pagnutti, S.

    2005-06-01

    We reconsider the derivation of semianalytical expressions providing the most significant aspects of the high-gain free-electron laser dynamics. We obtain new expressions for the growth of the laser power, of the e-beam-induced energy spread, and of the higher-order nonlinearly generated harmonics. The procedure we employ, based on theoretical ansatz and fitting methods, allows the determination of crucial quantities like the expected harmonic output power and its dependences on the e-beam parameters.

  4. Self-seeded FEL wavelength extension with high-gain harmonic generation

    NASA Astrophysics Data System (ADS)

    Zeng, Ling; Qin, Weilun; Zhao, Gang; Huang, Senlin; Ding, Yuantao; Huang, Zhirong; Marcus, Gabriel; Liu, Kexin

    2016-09-01

    We study a self-seeded high-gain harmonic generation (HGHG) free-electron laser (FEL) scheme to extend the wavelength of a soft X-ray FEL. This scheme uses a regular self-seeding monochromator to generate a seed laser at the wavelength of 1.52 nm, followed by a HGHG configuration to produce coherent, narrow-bandwidth harmonic radiations at the GW level. The 2nd and 3rd harmonic radiation is investigated with start-to-end simulations. Detailed studies of the FEL performance and shot-to-shot fluctuations are presented.

  5. EXPERIMENTAL DEMONSTRATION OF WAVELENGTH TUNING IN HIGH-GAIN HARMONIC GENERATION FREE ELECTRON LASER.

    SciTech Connect

    SHAFTAN,T.; JOHNSON,E.; KRINSKY,S.; LOOS,H.; MURPHY,J.B.; RAKOWSKY,G.; ROSE,J.; SHEEHY,B.; SKARITKA,J.; WANG,X.J.; WU,Z.; YU,L.H.

    2004-08-29

    Tunability is one of the key aspects of any laser system. In High-Gain Harmonic Generation Free Electron Laser (HGHG FEL) the seed laser determines the output wavelength. Conventional scheme of tunable HGHG FEL requires tunable seed laser. The alternative scheme [1] is based on compression of the electron bunch with energy-time correlation (chirped bunch) in the FEL dispersive section. The chirped energy modulation, induced by the seed laser with constant wavelength, compressed as the whole bunch undergoes compression. In this paper we discuss experimental verification of the proposed approach at the DUV FEL [2,3] and compare experimental results with analytical estimates.

  6. High-gain harmonic generation of soft X-rays with the `fresh bunch` technique

    SciTech Connect

    Yu, Li-Hua; Ben-Zvi, I.

    1996-10-01

    We report numerical simulations (using the TDA code) and analytic verification of the generation of 64 {Angstrom} high power soft X- rays from an exponential regime single pass seeded FEL. The seed is generated in the FEL using the High Gain Harmonic Generation (HGHG) technique combined with the `Fresh bunch` technique. A seed pulse at 2944 {Angstrom} is generated by conventional laser techniques. The seed pulse produces an intense energy modulation of the rear part of a I GeV, 1245 {Angstrom} electron beam in a `modulator` wiggler. In the `radiator` wiggler, (resonant to 64 {Angstrom}), the energy modulation creates beam density modulation followed by radiation of the 46{sup th} harmonic of the seed. We use a magnetic delay to position the 64 A{Angstrom} radiation at the undisturbed front of the bunch to serve as a seed for a single pass, exponential growth FEL. After a 9 m long exponential section followed by a 7 m long tapered section the radiation power reaches 3.3 GW.

  7. Oscillator Seeding of a High Gain Harmonic Generation FEL in a Radiator-First Configuration

    SciTech Connect

    Gandhi, P.; Wurtele, J.; Penn, G.; Reinsch, M.

    2012-05-20

    A longitudinally coherent X-ray pulse from a high repetition rate free electron laser (FEL) is desired for a wide variety of experimental applications. However, generating such a pulse with a repetition rate greater than 1 MHz is a significant challenge. The desired high repetition rate sources, primarily high harmonic generation with intense lasers in gases or plasmas, do not exist now, and, for the multi-MHz bunch trains that superconducting accelerators can potentially produce, are likely not feasible with current technology. In this paper, we propose to place an oscillator downstream of a radiator. The oscillator generates radiation that is used as a seed for a high gain harmonic generation (HGHG) FEL which is upstream of the oscillator. For the first few pulses the oscillator builds up power and, until power is built up, the radiator has no HGHG seed. As power in the oscillator saturates, the HGHG is seeded and power is produced. The dynamics and stability of this radiator-first scheme is explored analytically and numerically. A single-pass map is derived using a semi-analytic model for FEL gain and saturation. Iteration of the map is shown to be in good agreement with simulations. A numerical example is presented for a soft X-ray FEL.

  8. SOFT X-RAY FEL BY CASCADING STAGES OF HIGH GAIN HARMONIC GENERATION.

    SciTech Connect

    YU,L.H.

    2003-04-17

    Short wavelength Free-Electron Lasers are perceived as the next generation of synchrotron light sources. In the past decade, significant advances have been made in the theory and technology of high brightness electron beams and single pass FELs. These developments facilitate the construction of practical VUV FELs and make x-ray FELs possible. Self-Amplified Spontaneous Emission (SASE) and High Gain Harmonic Generation (HGHG)[17-19] are the two leading candidates for x-ray FELs. The first lasing of HGHG proof-of-principle experiment succeeded in August, 1999 in Brookhaven National Laboratory. The experimental results agree with the theory prediction. Compared with SASE FEL, the following advantages of HGHG FEL were confirmed; (1) Better longitudinal coherence, and hence, much narrower bandwidth than SASE. (2) More stable central wavelength, (3) More stable output energy. In this introduction, we will first briefly describe the principle of HGHG in Section A. Then in Section B, we give a general description about how to produce soft x-ray by cascading HGHG scheme. In section 2, we give a detailed description of the system design. Then, in section 3, we give a description of an analytical estimate for the HGHG process, and the calculation of the parameters of different parts of the system. The estimate is found to agree with simulation within about a factor 2 for most cases we studied. The stability issue, the sensitivity to parameter variation, the harmonic contents of the final output, and the noise degradation issue of such HGHG scheme are discussed in Section 4. The results are presented in Section 4. Finally, in Section 5, we will give some discussion of the challenges in development of the system. The conclusion is given in Section 6.

  9. Development of a 3D FEL code for the simulation of a high-gain harmonic generation experiment.

    SciTech Connect

    Biedron, S. G.

    1999-02-26

    Over the last few years, there has been a growing interest in self-amplified spontaneous emission (SASE) free-electron lasers (FELs) as a means for achieving a fourth-generation light source. In order to correctly and easily simulate the many configurations that have been suggested, such as multi-segmented wigglers and the method of high-gain harmonic generation, we have developed a robust three-dimensional code. The specifics of the code, the comparison to the linear theory as well as future plans will be presented.

  10. Study of the output pulse stability of a cascaded high-gain harmonic generation free-electron laser

    NASA Astrophysics Data System (ADS)

    Wang, Zhen; Feng, Chao; Gu, Qiang; Zhao, Zhentang

    2016-06-01

    Cascading stages of high-gain harmonic generation (HGHG) have been demonstrated to be a promising candidate for producing fully coherent soft X-ray radiation directly from UV seed sources. However, the large shot-to-shot output pulse energy fluctuation may still be a serious problem for its user applications. In this paper, we study the effects of various electron beam parameters jitters on the output pulse energy fluctuations of a two-stage HGHG. Theoretical calculations and intensive simulations have been performed and the results demonstrate that the relative timing jitter between the electron bunch and the seed laser pulse is mainly responsible for the large output pulse energy fluctuation. Several methods that may be helpful to improve the FEL stability have also been discussed.

  11. The Shanghai high-gain harmonic generation DUV free-electron laser

    NASA Astrophysics Data System (ADS)

    Zhao, Z. T.; Dai, Z. M.; Zhao, X. F.; Liu, D. K.; Zhou, Q. G.; He, D. H.; Jia, Q. K.; Chen, S. Y.; Dai, J. P.

    2004-08-01

    The Shanghai deep ultraviolet free-electron laser source (SDUV-FEL) is an HGHG FEL facility designed for generating coherent output with wavelength down to 88 nm. The design and the relevant R&D of this HGHG FEL source have been under way since 2000. Currently, a 150 MeV S-band electron injector is under construction as the first linac section to produce a high brightness beam. The design study and the present R&D status of the SDUV-FEL have been presented in this paper.

  12. Harmonic generation with multiple wiggler schemes

    SciTech Connect

    Bonifacio, R.; De Salvo, L.; Pierini, P.

    1995-02-01

    In this paper the authors give a simple theoretical description of the basic physics of the single pass high gain free electron laser (FEL), describing in some detail the FEL bunching properties and the harmonic generation technique with a multiple-wiggler scheme or a high gain optical klystron configuration.

  13. Higher harmonic generation microscopy.

    PubMed

    Sun, Chi-Kuang

    2005-01-01

    Higher harmonic-generation, including second harmonic generation and third harmonic generation, leaves no energy deposition to the interacted matters due to its virtual-level transition characteristic, providing a truly non-invasive modality and is ideal for in vivo imaging of live specimens without any preparation. Second harmonic generation microscopy provides images on stacked membranes and arranged proteins with organized nano-structures due to the bio-photonic crystalline effect. Third harmonic generation microscopy provides general cellular or subcellular interface imaging due to optical inhomogeneity. Due to their virtual-transition nature, no saturation or bleaching in the generated signal is expected. With no energy release, continuous viewing without compromising sample viability can thus be achieved. Combined with its nonlinearity, higher harmonic generation microscopy provides sub-micron three-dimensional sectioning capability and millimeter penetration in live samples without using fluorescence and exogenous markers, offering morphological, structural, functional, and cellular information of biomedical specimens without modifying their natural biological and optical environments.

  14. Optical harmonic generator

    DOEpatents

    Summers, Mark A.; Eimerl, David; Boyd, Robert D.

    1985-01-01

    A pair of uniaxial birefringent crystal elements are fixed together to form a serially arranged, integral assembly which, alternatively, provides either a linearly or elliptically polarized second-harmonic output wave or a linearly polarized third-harmonic output wave. The "extraordinary" or "e" directions of the crystal elements are oriented in the integral assembly to be in quadrature (90.degree.). For a second-harmonic generation in the Type-II-Type-II angle tuned case, the input fundamental wave has equal amplitude "o" and "e" components. For a third-harmonic generation, the input fundamental wave has "o" and "e" components whose amplitudes are in a ratio of 2:1 ("o":"e" reference first crystal). In the typical case of a linearly polarized input fundamental wave this can be accomplished by simply rotating the crystal assembly about the input beam direction by 10.degree.. For both second and third harmonic generation input precise phase-matching is achieved by tilting the crystal assembly about its two sensitive axes ("o").

  15. Optical harmonic generator

    DOEpatents

    Summers, M.A.; Eimerl, D.; Boyd, R.D.

    1982-06-10

    A pair of uniaxial birefringent crystal elements are fixed together to form a serially arranged, integral assembly which, alternatively, provides either a linearly or elliptically polarized second-harmonic output wave or a linearly polarized third-harmonic output wave. The extraordinary or e directions of the crystal elements are oriented in the integral assembly to be in quadrature (90/sup 0/). For a second-harmonic generation in the Type-II-Type-II angle tuned case, the input fundamental wave has equal amplitude o and e components. For a third-harmonic generation, the input fundamental wave has o and e components whose amplitudes are in a ratio of 2:1 (o:e reference first crystal). In the typical case of a linearly polarized input fundamental wave this can be accomplished by simply rotating the crystal assembly about the input beam direction by 10/sup 0/. For both second and third harmonic generation input precise phase-matching is achieved by tilting the crystal assembly about its two sensitive axeses (o).

  16. Nonlinear harmonic generation in distributed optical klystrons

    SciTech Connect

    H.P. Freund; George R. Neil

    2001-12-01

    A distributed optical klystron has the potential for dramatically shortening the total interaction length in high-gain free-electron lasers (INP 77-59, Novosibirsk, 1977; Nucl. Instr. and Meth A 304 (1991) 463) in comparison to a single-wiggler-segment configuration. This shortening can be even more dramatic if a nonlinear harmonic generation mechanism is used to reach the desired wavelength. An example operating at a 4.5{angstrom} fundamental and a 1.5{angstrom} harmonic is discussed.

  17. Design of a high-power, high-gain, 2nd harmonic, 22.848 GHz gyroklystron

    SciTech Connect

    Veale, M.; Purohit, P.; Lawson, W.

    2013-08-15

    In this paper we consider the design of a four-cavity, high-gain K-band gyroklystron experiment for high gradient structure testing. The frequency doubling gyroklystron utilizes a beam voltage of 500 kV and a beam current of 200 A from a magnetron injection gun (MIG) originally designed for a lower-frequency device. The microwave circuit features input and gain cavities in the circular TE{sub 011} mode and penultimate and output cavities that operate at the second harmonic in the TE{sub 021} mode. We investigate the MIG performance and study the behavior of the circuit for different values of perpendicular to parallel velocity ratio (α= V{sub ⊥}/ V{sub z}). This microwave tube is expected to be able to produce at least 20 MW of power in 1μs pulses at a repetition rate of at least 120 Hz. A maximum efficiency of 26% and a large signal gain of 58 dB under zero-drive stable conditions were simulated for a velocity ratio equal to 1.35.

  18. Nonlinear harmonic generation in the STARS FEL

    NASA Astrophysics Data System (ADS)

    Abo-Bakr, M.; Goldammer, K.; Kamps, T.; Knobloch, J.; Kuske, B.; Leitner, T.; Meseck, A.

    2008-08-01

    BESSY proposes to build STARS, an FEL to demonstrate cascaded High Gain Harmonic Generation (HGHG). In two HGHG stages, a laser source of 700-900 nm is converted down to a wavelength of 40-70 nm. The STARS facility consists of a normal-conducting RF photoinjector, three superconducting TESLA-type acceleration modules, a magnetic bunch compressor and two stages of HGHG, each consisting of a modulator, dispersive chicane and a radiator. At the entrance of the undulator section, the beam energy is 325 MeV and the peak current is about 500 A. With these parameters, the STARS FEL reaches saturation with a peak power of 100-350 MW. A superradiant mode is also foreseen which boosts the radiation power to the GW-level. Due to nonlinear harmonic generation (NHG), free electron lasers also radiate coherently at higher harmonics of the FEL resonant frequency. STARS can hence extend its output range to even shorter wavelengths. This paper presents studies of the STARS harmonic content in the wavelength range of 6-20 nm. Seeding with high harmonic generation pulses at 32 nm is also discussed.

  19. Echo-Enabled Harmonic Generation

    SciTech Connect

    Stupakov, Gennady; /SLAC

    2012-06-28

    A recently proposed concept of the Echo-Enabled Harmonic Generation (EEHG) FEL uses two laser modulators in combination with two dispersion sections to generate a high-harmonic density modulation in a relativistic beam. This seeding technique holds promise of a one-stage soft x-ray FEL that radiates not only transversely but also longitudinally coherent pulses. Currently, an experimental verification of the concept is being conducted at the SLAC National Accelerator Laboratory aimed at the demonstration of the EEHG.

  20. Echo-Enabled Harmonic Generation

    SciTech Connect

    Stupakov, Gennady

    2010-08-25

    A recently proposed concept of the Echo-Enabled Harmonic Generation (EEHG) FEL uses two laser modulators in combination with two dispersion sections to generate a high-harmonic density modulation in a relativistic beam. This seeding technique holds promise of a one-stage soft x-ray FEL that radiates not only transversely but also longitudinally coherent pulses. Currently, an experimental verification of the concept is being conducted at the SLAC National Accelerator Laboratory aimed at the demonstration of the EEHG.

  1. Dislocation Detection Through Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Reinhardt, B. T.; Kropf, M.; Boudraeu, K.; Guers, M. J.; Tittmann, B. R.

    2010-02-01

    A fundamental goal of ultrasonic nondestructive evaluation is to characterize material defects before failure. During material fatigue, dislocations tend to nucleate, becoming sources of stress concentration. Eventually, cracks start to form and lead to material failure. Recent research has indicated that nonlinear harmonic generation can be used to distinguish between materials of high and low dislocation densities. This research reports nonlinear harmonic generation measurements to distinguish between those areas of high and low dislocation densities in copper bars. The copper bars were subjected to flexural fatigue. Periodic scans were taken in order to track dislocation development during the fatigue life of the material. We show that this technique provides improved early detection for critical components of failure.

  2. Organometallic Salts Generate Optical Second Harmonics

    NASA Technical Reports Server (NTRS)

    Marder, Seth R.; Perry, Joseph W.

    1991-01-01

    Series of organometallic salts exhibit large second-order dielectric susceptibilities, as evidenced by generation of second harmonics when illuminated at visible and near-infrared wavelengths. Investigations of these and related compounds continue with view toward development of materials for use as optical second-harmonic generators, electro-optical modulators, optical switches, piezoelectric sensors, and parametric crystals.

  3. Resonantly-enhanced harmonic generation in Argon.

    PubMed

    Ackermann, P; Münch, H; Halfmann, T

    2012-06-18

    We present systematic investigations of harmonic generation in Argon, driven in the vicinity of a five-photon resonance by intense, tunable picosecond radiation pulses. When properly matching the laser frequency with the Stark-shifted multi-photon resonance, we observe a pronounced enhancement not only of the 5th, but also the 7th and 9th harmonic of the driving laser (i.e. at orders higher than the involved multi-photon resonance). We study the harmonic yield at different intensities and wavelengths of the driving laser to determine optimal conditions for resonantly-enhanced harmonic generation.

  4. Harmonic generation in magnetized quantum plasma

    NASA Astrophysics Data System (ADS)

    Kumar, Punit; Singh, Shiv; Singh, Abhisek Kumar

    2016-05-01

    A study of second harmonic generation by propagation of a linearly polarized electromagnetic wave through homogeneous high density quantum plasma in the presence of transverse magnetic field. The nonlinear current density and dispersion relations for the fundamental and second harmonic frequencies have been obtained using the recently developed quantum hydrodynamic (QHD) model. The effect of quantum Bohm potential, Fermi pressure and the electron spin have been taken into account. The second harmonic is found to be less dispersed than the first.

  5. Surface-Enhanced Second-Harmonic Generation

    SciTech Connect

    Chen, C. K.; de Castro, A. R.B.; Shen, Y. R.

    1981-01-12

    Second harmonic generation at a silver-air interface was enhanced due to surface roughness by a factor of 10⁴. The local field enhancement is believed to be responsible for the effect. An unusually broad luminescence background extending far beyond the antiStokes side of the second harmonic was also observed.

  6. High order harmonic generation in rare gases

    SciTech Connect

    Budil, K.S.

    1994-05-01

    The process of high order harmonic generation in atomic gases has shown great promise as a method of generating extremely short wavelength radiation, extending far into the extreme ultraviolet (XUV). The process is conceptually simple. A very intense laser pulse (I {approximately}10{sup 13}-10{sup 14} W/cm{sup 2}) is focused into a dense ({approximately}10{sup l7} particles/cm{sup 3}) atomic medium, causing the atoms to become polarized. These atomic dipoles are then coherently driven by the laser field and begin to radiate at odd harmonics of the laser field. This dissertation is a study of both the physical mechanism of harmonic generation as well as its development as a source of coherent XUV radiation. Recently, a semiclassical theory has been proposed which provides a simple, intuitive description of harmonic generation. In this picture the process is treated in two steps. The atom ionizes via tunneling after which its classical motion in the laser field is studied. Electron trajectories which return to the vicinity of the nucleus may recombine and emit a harmonic photon, while those which do not return will ionize. An experiment was performed to test the validity of this model wherein the trajectory of the electron as it orbits the nucleus or ion core is perturbed by driving the process with elliptically, rather than linearly, polarized laser radiation. The semiclassical theory predicts a rapid turn-off of harmonic production as the ellipticity of the driving field is increased. This decrease in harmonic production is observed experimentally and a simple quantum mechanical theory is used to model the data. The second major focus of this work was on development of the harmonic {open_quotes}source{close_quotes}. A series of experiments were performed examining the spatial profiles of the harmonics. The quality of the spatial profile is crucial if the harmonics are to be used as the source for experiments, particularly if they must be refocused.

  7. High-harmonic generation in cavitated plasmas

    SciTech Connect

    Schroeder, C. B.; Esarey, E.; Comier-Michel, E.; Leemans, W. P.

    2008-05-15

    A method is proposed for producing coherent x-rays via high-harmonic generation using ultraintense lasers interacting with highly stripped ions in cavitated plasmas. This method relies on plasma cavitation by the wake of an intense drive beam (laser or electron beam) to produce an ion cavity. An ultrashort pulse laser propagating in the plasma-electron-free ion cavity generates laser harmonics. The longitudinal electron motion, which inhibits high-harmonic generation at high laser intensities, can be suppressed by the space-charge field in the ion cavity or by using a counterpropagating laser pulse. Periodic suppression of the longitudinal electron motion may also be used to quasi-phase-match. This method enables harmonic generation to be extended to the sub-A regime.

  8. Echo-Enabled Harmonic Generation for Seeded FELs

    SciTech Connect

    Stupakov, G.; /SLAC

    2011-05-19

    In the x-ray wavelengths, the two leading FEL concepts are the self-amplified spontaneous emission (SASE) configuration and the high-gain harmonic generation (HGHG) scheme. While the radiation from a SASE FEL is coherent transversely, it typically has rather limited temporal coherence. Alternatively, the HGHG scheme allows generation of fully coherent radiation by up-converting the frequency of a high-power seed laser. However, due to the relatively low up-frequency conversion efficiency, multiple stages of HGHG FEL are needed in order to generate x-rays from a UV laser. The up-frequency conversion efficiency can be greatly improved with the recently proposed echo-enabled harmonic generation (EEHG) technique. In this work we will present the concept of EEHG, and address some practically important issues that affect the performance of the seeding. We show how the EEHG can be incorporated in the FEL scheme and what is the expected performance of the EEHG seeded FEL. We will then briefly describe the first proof-of-principle EEHG experiment carried out at the Next Linear Collider Test Accelerator (NLCTA) at SLAC. We will also discuss latest advances in the echo-scheme approach, and refer to subsequent modifications of the original concept.

  9. Microwave harmonic generation and nonlinearity in microplasmas

    NASA Astrophysics Data System (ADS)

    Gregório, José; Parsons, Stephen; Hopwood, Jeffrey

    2016-06-01

    Nonlinearities in microplasmas excited by microwaves are described both experimentally and through a 2D fluid model. A split-ring resonator generates a microplasma in a 150 μm discharge gap at 1 GHz. Nonlinearity generates both radiated and conducted harmonics which are measured from 0.2–760 Torr (Ar) for power levels between 0.5 and 3 W. Asymmetric electrode configurations produce the highest 3rd harmonic power (>10 mW) at an optimal pressure of the order of 0.3 Torr. The microplasma is also demonstrated as a mixer. The experimental results are explained with the aid of a fluid model of the microplasma. The model shows that the smaller electrode in an asymmetric device is forced to attain a large microwave potential that strongly modulates the sheath thickness and the local electron energy. The voltage-dependent sheath width gives rises to a nonlinear sheath capacitance as well as short pulses of hot electron flux to the electrode. The modeled 3rd harmonic current is converted to an extractable harmonic power by a microwave circuit model. Using this technique the modeled and measured harmonic production of the microplasma are found to compare favorably.

  10. Generation of GW-Level, Sub-Angstrom Radiation in the LCLS Using a Second-Harmonic Radiator

    SciTech Connect

    Huang, Z

    2004-09-14

    Electron beams are strongly microbunched near the high-gain free-electron laser (FEL) saturation with a rich harmonic content in the beam current. While the coherent harmonic emission is possible in a planar undulator, the third-harmonic radiation typically dominates with about 1% of the fundamental power at saturation. In this paper, we discuss the second-harmonic radiation in the Linac Coherent Light Source. We show that by a suitable design of an second-stage undulator with its fundamental frequency tuned to the second harmonic of the first undulator, coherent second-harmonic radiation much more intense than the third-harmonic is emitted. Numerical simulations predict that GW-level, sub-Angstrom x-ray pulses can be generated in a relatively short second-harmonic radiator.

  11. Inhomogeneous high harmonic generation in krypton clusters.

    PubMed

    Ruf, H; Handschin, C; Cireasa, R; Thiré, N; Ferré, A; Petit, S; Descamps, D; Mével, E; Constant, E; Blanchet, V; Fabre, B; Mairesse, Y

    2013-02-22

    High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from monomers and clusters is challenging. By performing a spectrally and spatially resolved study in a controlled mixture of clusters and monomers, we are able to isolate a region of the spectrum where the emission purely originates from clusters. Surprisingly, the emission from clusters is depolarized, which is the signature of statistical inhomogeneous emission from a low-density source. The harmonic response to laser ellipticity shows that this generation is produced by a new recollisional mechanism, which opens the way to future theoretical studies.

  12. Fast interferometric second harmonic generation microscopy

    PubMed Central

    Bancelin, Stéphane; Couture, Charles-André; Légaré, Katherine; Pinsard, Maxime; Rivard, Maxime; Brown, Cameron; Légaré, François

    2016-01-01

    We report the implementation of fast Interferometric Second Harmonic Generation (I-SHG) microscopy to study the polarity of non-centrosymmetric structures in biological tissues. Using a sample quartz plate, we calibrate the spatially varying phase shift introduced by the laser scanning system. Compensating this phase shift allows us to retrieve the correct phase distribution in periodically poled lithium niobate, used as a model sample. Finally, we used fast interferometric second harmonic generation microscopy to acquire phase images in tendon. Our results show that the method exposed here, using a laser scanning system, allows to recover the polarity of collagen fibrils, similarly to standard I-SHG (using a sample scanning system), but with an imaging time about 40 times shorter. PMID:26977349

  13. High-order harmonic generation in alkanes

    SciTech Connect

    Altucci, C.; Velotta, R.; Heesel, E.; Springate, E.; Marangos, J. P.; Vozzi, C.; Benedetti, E.; Calegari, F.; Sansone, G.; Stagira, S.; Nisoli, M.; Tosa, V.

    2006-04-15

    We have investigated the process of high-order harmonic generation in light alkanes by using femtosecond laser pulses. We show the experimental results cannot be matched by a model that assumes a single active electron only in a hydrogenic s orbital. Clear evidences are shown of the important role played by the p-like character originating from the covalent C-H bond. By constructing a suitable mixture of s-type and p-type atomic wave functions, an excellent agreement between measurements in methane and simulations is found, thus confirming the validity of the developed method as a general tool for the analysis of high-order harmonic generation in complex molecules.

  14. Generating Second Harmonics In Nonlinear Resonant Cavities

    NASA Technical Reports Server (NTRS)

    Kozlovsky, William J.; Nabors, C. David; Byer, Robert L.

    1990-01-01

    Single-axial-mode lasers pump very-low-loss doubling crystals. Important advance in making resonant generation of second harmonics possible for diode-laser-pumped solid-state lasers is recent development of monolithic nonplanar ring geometries in neodymium:yttrium aluminum garnet (Nd:YAG) lasers that produce frequency-stable single-mode outputs. Other advance is development of high-quality MgO:LiNbO3 as electro-optically nonlinear material. Series of experiments devised to improve doubling efficiency of low-power lasers, and particularly of diode-laser-pumped continuous-wave Nd:YAG lasers.

  15. High harmonic generation in undulators for FEL

    NASA Astrophysics Data System (ADS)

    Zhukovsky, K.

    2016-02-01

    The analytical study of the undulator radiation (UR), accounting for major sources of the spectral line broadening is presented. Analytical expressions for the UR spectrum and intensity are obtained. They demonstrate possibilities of the compensation of the divergency by the constant magnetic component. Some examples of single and double frequency undulators are considered. Generation of harmonics is studied with account for homogeneous and inhomogeneous broadening in real devices. The obtained results with account for all broadening sources are applied for evaluation of free electron laser (FEL) performance and compared with those, obtained with the ideal undulator.

  16. Promoting Spontaneous Second Harmonic Generation through Organogelation.

    PubMed

    Marco, A Belén; Aparicio, Fátima; Faour, Lara; Iliopoulos, Konstantinos; Morille, Yohann; Allain, Magali; Franco, Santiago; Andreu, Raquel; Sahraoui, Bouchta; Gindre, Denis; Canevet, David; Sallé, Marc

    2016-07-27

    An organogelator based on the Disperse Red nonlinear optical chromophore was synthesized according to a simple and efficient three-step procedure. The supramolecular gel organization leads to xerogels which display a spontaneous second harmonic generation (SHG) response without any need for preprocessing, and this SHG activity appears to be stable over several months. These findings, based on an intrinsic structural approach, are supported by favorable intermolecular supramolecular interactions, which promote a locally non-centrosymmetric NLO-active organization. This is in sharp contrast with most materials designed for SHG purposes, which generally require the use of expensive or heavy-to-handle external techniques for managing the dipoles' alignment. PMID:27415660

  17. Limitations and improvements for harmonic generation measurements

    SciTech Connect

    Best, Steven; Croxford, Anthony; Neild, Simon

    2014-02-18

    A typical acoustic harmonic generation measurement comes with certain limitations. Firstly, the use of the plane wave-based analysis used to extract the nonlinear parameter, β, ignores the effects of diffraction, attenuation and receiver averaging which are common to most experiments, and may therefore limit the accuracy of a measurement. Secondly, the method usually requires data obtained from a through-transmission type setup, which may not be practical in a field measurement scenario where access to the component is limited. Thirdly, the technique lacks a means of pinpointing areas of damage in a component, as the measured nonlinearity represents an average over the length of signal propagation. Here we describe a three-dimensional model of harmonic generation in a sound beam, which is intended to provide a more realistic representation of a typical experiment. The presence of a reflecting boundary is then incorporated into the model to assess the feasibility of performing single-sided measurements. Experimental validation is provided where possible. Finally, a focusing acoustic source is modelled to provide a theoretical indication of the afforded advantages when the nonlinearity is localized.

  18. Helicopter high gain control

    NASA Technical Reports Server (NTRS)

    Cunningham, T. B.; Nunn, E. C.

    1979-01-01

    High gain control is explored through a design study of the CH-47B helicopter. The plans are designed to obtain the maximum bandwidth possible given the hardware constraints. Controls are designed with modal control theory to specific bandwidths and closed loop mode shapes. Comparisons are made to an earlier complementary filter approach. Bandwidth improvement by removal of limitations is explored in order to establish hardware and mechanization options. Improvements in the pitch axis control system and in the rate gyro sensor noise characteristics in all axes are discussed. The use of rotor state feedback is assessed.

  19. Collapsible high gain antenna

    NASA Technical Reports Server (NTRS)

    Cribb, H. E. (Inventor)

    1973-01-01

    A lightweight small high gain antenna which is capable of being packaged in a collapsed form and automatically expanded when in use is described. The antenna includes a cylindrical housing having a rod with a piston adjacent to one end extending through it. Attached to the outer end of the rod in a normally collapsed state is a helical wire coil. When the gas producing means is activated the piston and rod are shifted outwardly to expand the wire coil. A latch is provided for holding the helical coil in the expanded position.

  20. Orientation dependence of high-order harmonic generation in molecules

    NASA Astrophysics Data System (ADS)

    Lein, M.; Corso, P. P.; Marangos, J. P.; Knight, P. L.

    2003-02-01

    We present two- and three-dimensional model calculations of high-order harmonic generation in H+2. The harmonic spectra exhibit clear signatures of intramolecular interference. An interference minimum appears at a harmonic order that depends on the molecular orientation. Harmonic generation in three-center molecules is studied on the basis of two-dimensional calculations for a H2+3 model system. From analytical considerations, the orientation dependence of the harmonic intensities in three-center molecules exhibits a double minimum due to intramolecular interference. In the numerical results, the double minimum is broadened into a single wide minimum. The effect of nonzero laser ellipticity on harmonic generation is investigated by means of two-dimensional simulations for H+2. We find that harmonic generation with elliptical polarization is governed by interference effects similar to linear polarization.

  1. Modelling harmonic generation measurements in solids.

    PubMed

    Best, S R; Croxford, A J; Neild, S A

    2014-02-01

    Harmonic generation measurements typically make use of the plane wave result when extracting values for the nonlinearity parameter, β, from experimental measurements. This approach, however, ignores the effects of diffraction, attenuation, and receiver integration which are common features in a typical experiment. Our aim is to determine the importance of these effects when making measurements of β over different sample dimensions, or using different input frequencies. We describe a three-dimensional numerical model designed to accurately predict the results of a typical experiment, based on a quasi-linear assumption. An experiment is designed to measure the axial variation of the fundamental and second harmonic amplitude components in an ultrasonic beam, and the results are compared with those predicted by the model. The absolute β values are then extracted from the experimental data using both the simulation and the standard plane wave result. A difference is observed between the values returned by the two methods, which varies with axial range and input frequency. PMID:23786784

  2. Harmonic generation by circularly polarized laser beams propagating in plasma

    SciTech Connect

    Agrawal, Ekta; Hemlata,; Jha, Pallavi

    2015-04-15

    An analytical theory is developed for studying the phenomenon of generation of harmonics by the propagation of an obliquely incident, circularly polarized laser beam in homogeneous, underdense plasma. The amplitudes of second and third harmonic radiation as well as detuning distance have been obtained and their variation with the angle of incidence is analyzed. The amplitude of harmonic radiation increases with the angle of incidence while the detuning distance decreases, for a given plasma electron density. It is observed that the generated second and third harmonic radiation is linearly and elliptically polarized, respectively. The harmonic radiation vanishes at normal incidence of the circularly polarized laser beam.

  3. Goos-Hänchen shifts in harmonic generation from metals.

    PubMed

    Yallapragada, V J; Gopal, Achanta Venu; Agarwal, G S

    2013-05-01

    We present the first calculation of the Goos-Hänchen shifts in the context of the nonlinear generation of fields. We specifically concentrate on shifts of second harmonic generated at metallic surfaces. At metallic surfaces the second harmonic primarily arises from discontinuities of the field at surfaces which not only result in large harmonic generation but also in significant Goos-Hänchen shifts of the generated second harmonic. Our results can be extended to other shifts like angular shifts and Fedorov-Imbert shifts.

  4. Generation mechanism of power line harmonic radiation

    NASA Astrophysics Data System (ADS)

    Kostrov, Alexander; Gushchin, Mikhail; Korobkov, Sergei

    The questions concerning the generation of power line harmonic radiation (PLHR) and magne-tospheric line radiation (MLR) are discussed, including the effective source of high harmonics of 50/60 Hz, and fine dynamic structure of the frequency spectrum of PLHR and MLR. It is shown, that thyristor-based power regulators used by large electrical power consumers produce the periodic sequences of current pulses with duration of about 10 microseconds in a power line. The repetition rate of these pulses is typically 100/120 Hz; the bandwidth is as broad as 100 kHz. For high harmonics of 50/60 Hz, the power line represents an effective traveling-wave (or Beverage) antenna, especially in a frequency range of several kHz corresponding to VLF whistler band in Earth ionosphere and magnetosphere. For the fixed length of the power line, which acts as antenna, radiation directivity diagram in relation to horizon depends of frequency. Hence the spatial separation of whistlers emitted at various frequencies (1-10 kHz in a consid-ered case) is possible, with subsequent propagation of whistlers with different frequencies along different L-shells. Estimations show that the efficiency of power line as travelling-wave antenna can be changed by variations of its load, but not more than twice ("weekend effect"). Since the PLHR can represent the sequence of short electromagnetic bursts, then careful se-lection of frequency-time resolution of the data acquisition equipment is needed. Typically, the time constant of the data recording and processing is too large, and the spectra of PLHR or MLR are characterized by a well-known line structure. At the same time, original bursty structure of PLHR can not be defined. Fine structure of MLR is also discussed. Frequency drift of MLR can be explained by the perturbations of the magnetospheric plasma by intense ULF waves and particle flows affecting the propagation of PLHR. Hence the physical nature of PLHR and MLR is the same, excepting the

  5. Origin of second-harmonic generation from individual silicon nanowires

    NASA Astrophysics Data System (ADS)

    Wiecha, Peter R.; Arbouet, Arnaud; Girard, Christian; Baron, Thierry; Paillard, Vincent

    2016-03-01

    We investigate second harmonic generation from individual silicon nanowires and study the influence of resonant optical modes on the far field nonlinear emission. We find that the polarization of the second harmonic has a size-dependent behavior and explain this phenomenon by considering different surface and bulk nonlinear susceptibility contributions. We show that the second harmonic generation has an entirely different origin, depending on the nanowire diameter and on whether the incident illumination is polarized parallel or perpendicular to the nanowire axis. The results open perspectives for further geometry-based studies on the origin and control of second harmonic generation in nanostructures of high-refractive index centrosymmetric dielectrics.

  6. Miniaturized Blue Laser using Second Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Kitaoka, Yasuo; Yokoyama, Toshifumi; Mizuuchi, Kiminori; Yamamoto, Kazuhisa

    2000-06-01

    We demonstrate a miniaturized blue laser (5× 12× 1.5 mm3) using second harmonic generation (SHG), which consists of a quasi-phase-matched (QPM)-SHG waveguide device on an x-cut Mg-doped LiNbO3 substrate and a tunable distributed-Bragg-reflector (DBR) laser diode. By using the QPM-SHG waveguide device on an x-cut substrate, efficient optical coupling was realized without a half-wave plate, and the maximum coupling efficiency of 75% was achieved. The blue light power of 2 mW was generated for the fundamental coupling power of 20 mW, which agreed with a conversion efficiency of 10%. The mechanical stability of the planar-type butt-coupled SHG blue laser was examined, where the coupling efficiency was maintained constantly under the change of module temperature and the temperature cycle test from 10 to 60°C. We succeeded in downsizing the SHG blue laser to 0.1 cm3, which is sufficiently small for its application to optical disk systems.

  7. A superconducting short period undulator for a harmonic generation FEL experiment

    SciTech Connect

    Ingold, G.; Solomon, L.; Ben-Zvi, I.; Krinsky, S.; Li, D.; Lynch, D.; Sheehan, J.; Woodle, M.; Qiu, X.Z.; Yu, L.H.; Zhang, X.; Sampson, W.; Gardner, M.; Robins, K.; Lehrman, I.; Heuer, R.; Sheehan, J.; Weissenburger, D.

    1993-07-01

    A three stage superconducting (SC) undulator for a high gain harmonic generation (HGE) FEL experiment in the infrared is under construction at the NSLS in collaboration with Grumman Corporation. A novel undulator technology suitable for short period (6--40mm) undulators will be employed for all three stages, the modulator, the dispersive section and the radiator. The undulator triples the frequency of a 10.4{mu}m CO{sub 2} seed laser. So far a 27 period (one third of the final radiator) prototype radiator has been designed, built and tested.

  8. A superconducting short period undulator for a harmonic generation FEL experiment

    SciTech Connect

    Ingold, G.; Solomon, L.; Ben-Zvi, I.; Krinsky, S.; Li, D.; Lynch, D.; Sheehan, J.; Woodle, M.; Qiu, X.Z.; Yu, L.H.; Zhang, X.; Sampson, W.; Gardner, M.; Robins, K. ); Lehrman, I.; Heuer, R.; Sheehan, J.; Weissenburger, D. )

    1993-01-01

    A three stage superconducting (SC) undulator for a high gain harmonic generation (HGE) FEL experiment in the infrared is under construction at the NSLS in collaboration with Grumman Corporation. A novel undulator technology suitable for short period (6--40mm) undulators will be employed for all three stages, the modulator, the dispersive section and the radiator. The undulator triples the frequency of a 10.4[mu]m CO[sub 2] seed laser. So far a 27 period (one third of the final radiator) prototype radiator has been designed, built and tested.

  9. Intense harmonics generation with customized photon frequency and optical vortex

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaomei; Shen, Baifei; Shi, Yin; Zhang, Lingang; Ji, Liangliang; Wang, Xiaofeng; Xu, Zhizhan; Tajima, Toshiki

    2016-08-01

    An optical vortex with orbital angular momentum (OAM) enriches the light and matter interaction process, and helps reveal unexpected information in relativistic nonlinear optics. A scheme is proposed for the first time to explore the origin of photons in the generated harmonics, and produce relativistic intense harmonics with expected frequency and an optical vortex. When two counter-propagating Laguerre-Gaussian laser pulses impinge on a solid thin foil and interact with each other, the contribution of each input pulse in producing harmonics can be distinguished with the help of angular momentum conservation of photons, which is almost impossible for harmonic generation without an optical vortex. The generation of tunable, intense vortex harmonics with different photon topological charge is predicted based on the theoretical analysis and three-dimensional particle-in-cell simulations. Inheriting the properties of OAM and harmonics, the obtained intense vortex beam can be applied in a wide range of fields, including atom or molecule control and manipulation.

  10. Intense harmonics generation with customized photon frequency and optical vortex

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaomei; Shen, Baifei; Shi, Yin; Zhang, Lingang; Ji, Liangliang; Wang, Xiaofeng; Xu, Zhizhan; Tajima, Toshiki

    2016-08-01

    An optical vortex with orbital angular momentum (OAM) enriches the light and matter interaction process, and helps reveal unexpected information in relativistic nonlinear optics. A scheme is proposed for the first time to explore the origin of photons in the generated harmonics, and produce relativistic intense harmonics with expected frequency and an optical vortex. When two counter-propagating Laguerre–Gaussian laser pulses impinge on a solid thin foil and interact with each other, the contribution of each input pulse in producing harmonics can be distinguished with the help of angular momentum conservation of photons, which is almost impossible for harmonic generation without an optical vortex. The generation of tunable, intense vortex harmonics with different photon topological charge is predicted based on the theoretical analysis and three-dimensional particle-in-cell simulations. Inheriting the properties of OAM and harmonics, the obtained intense vortex beam can be applied in a wide range of fields, including atom or molecule control and manipulation.

  11. Second harmonic generation in human ovarian neoplasias

    NASA Astrophysics Data System (ADS)

    Lamonier, L.; Bottcher-Luiz, F.; Pietro, L.; Andrade, L. A. L. A.; de Thomaz, A. A.; Machado, C. L.; Cesar, C. L.

    2010-02-01

    Metastasis is the main cause of death in cancer patients; it requires a complex process of tumor cell dissemination, extra cellular matrix (ECM) remodeling, cell invasion and tumor-host interactions. Collagen is the major component of ECM; its fiber polymerization or degradation evolves in parallel with the evolution of the cancerous lesions. This study aimed to identify the collagen content, spatial distribution and fiber organization in biopsies of benign and malignant human ovarian tissues. Biopsies were prepared in slides without dyes and were exposed to 800nm Ti:Sapphire laser (Spectra Physics, 100 fs pulse duration, 800mW average power, 80MHz repetition rate). The obtained images were recorded at triplets, corresponding to clear field, multiphoton and second harmonic generation (SHG) mycroscopy. Data showed considerable anisotropy in malignant tissues, with regions of dense collagen arranged as individual fibers or in combination with immature segmental filaments. Radial fiber alignment or regions with minimal signal were observed in the high clinical grade tumors, suggesting degradation of original fibers or altered polymerization state of them. These findings allow us to assume that the collagen signature will be a reliable and a promising marker for diagnosis and prognosis in human ovarian cancers.

  12. Second harmonic generation from the 'centrosymmetric' crystals.

    PubMed

    Nalla, Venkatram; Medishetty, Raghavender; Wang, Yue; Bai, Zhaozhi; Sun, Handong; Wei, Ji; Vittal, Jagadese J

    2015-05-01

    Second harmonic generation (SHG) is a well known non-linear optical phenomena which can be observed only in non-centrosymmetric crystals due to non-zero hyperpolarizability. In the current work we observed SHG from a Zn(II) complex which was originally thought to have crystallized in the centrosymmetric space group C2/c. This has been attributed to the unequal antiparallel packing of the metal complexes in the non-symmetric space group Cc or residual non-centrosymmetry in C2/c giving rise to polarizability leading to strong SHG. The enhancement of SHG by UV light has been attributed to the increase in non-centrosymmetry and hence polarity of packing due to strain induced in the crystals. The SHG signals measured from these crystals were as large as potassium dihydrogen phosphate crystals, KH2PO4 (KDP), and showed temperature dependence. The highest SHG efficiency was observed at 50 K. The SHG phenomenon was observed at broad wavelengths ranging from visible to below-red in these crystals.

  13. Second harmonic generation polarization properties of myofilaments

    NASA Astrophysics Data System (ADS)

    Samim, Masood; Prent, Nicole; Dicenzo, Daniel; Stewart, Bryan; Barzda, Virginijus

    2014-05-01

    Second harmonic generation (SHG) polarization microscopy was used to investigate the organization of myosin nanomotors in myofilaments of muscle cells. The distribution of the second-order nonlinear susceptibility component ratio χzzz(2)/χzxx(2) along anisotropic bands of sarcomeres revealed differences between the headless and head-containing regions of myofilaments. The polarization-in polarization-out SHG measurements of headless myosin mutants of indirect flight muscle in Drosophila melanogaster confirmed a lower susceptibility component ratio compared to the head-containing myocytes with wild-type myosins. The increase in the ratio is assigned to the change in the deflection angle of the myosin S2 domain and possible contribution of myosin heads. The nonlinear susceptibility component ratio is a sensitive indicator of the myosin structure, and therefore, it can be used for conformational studies of myosin nanomotors. The measured ratio values can also be used as the reference for ab initio calculations of nonlinear optical properties of different parts of myosins.

  14. Higher-Order Harmonic Generation from Fullerene by Means of the Plasma Harmonic Method

    SciTech Connect

    Ganeev, R. A.; Bom, L. B. Elouga; Abdul-Hadi, J.; Ozaki, T.; Wong, M. C. H.; Brichta, J. P.; Bhardwaj, V. R.

    2009-01-09

    We demonstrate, for the first time, high-order harmonic generation from C{sub 60} by an intense femtosecond Ti:sapphire laser. Laser-produced plasmas from C{sub 60}-rich epoxy and C{sub 60} films were used as the nonlinear media. Harmonics up to the 19th order were observed. The harmonic yield from fullerene-rich plasma is about 25 times larger compared with those produced from a bulk carbon target. Structural studies of plasma debris confirm the presence and integrity of fullerenes within the plasma plume, indicating fullerenes as the source of high-order harmonics.

  15. Nonlinear harmonic generation and proposed experimental verification in SASE FELs.

    SciTech Connect

    Biedron, S. G.; Freund, H. P.; Milton, S. V.

    1999-08-24

    Recently, a 3D, polychromatic, nonlinear simulation code was developed to study the growth of nonlinear harmonics in self-amplified spontaneous emission (SASE) free-electron lasers (FELs). The simulation was applied to the parameters for each stage of the Advanced Photon Source (APS) SASE FEL, intended for operation in the visible, UV, and short UV wavelength regimes, respectively, to study the presence of nonlinear harmonic generation. Significant nonlinear harmonic growth is seen. Here, a discussion of the code development, the APS SASE FEL, the simulations and results, and, finally, the proposed experimental procedure for verification of such nonlinear harmonic generation at the APS SASE FEL will be given.

  16. Second-harmonic generation with Bessel beams

    NASA Astrophysics Data System (ADS)

    Shatrovoy, Oleg

    We present the results of a numerical simulation tool for modeling the second-harmonic generation (SHG) interaction experienced by a diffracting beam. This code is used to study the simultaneous frequency and spatial profile conversion of a truncated Bessel beam that closely resembles a higher-order mode (HOM) of an optical fiber. SHG with Bessel beams has been investigated in the past and was determined have limited value because it is less efficient than SHG with a Gaussian beam in the undepleted pump regime. This thesis considers, for the first time to the best of our knowledge, whether most of the power from a Bessel-like beam could be converted into a second-harmonic beam (full depletion), as is the case with a Gaussian beam. We study this problem because using HOMs for fiber lasers and amplifiers allows reduced optical intensities, which mitigates nonlinearities, and is one possible way to increase the available output powers of fiber laser systems. The chief disadvantage of using HOM fiber amplifiers is the spatial profile of the output, but this can be transformed as part of the SHG interaction, most notably to a quasi-Gaussian profile when the phase mismatch meets the noncollinear criteria. We predict, based on numerical simulation, that noncollinear SHG (NC-SHG) can simultaneously perform highly efficient (90%) wavelength conversion from 1064 nm to 532 nm, as well as concurrent mode transformation from a truncated Bessel beam to a Gaussian-like beam (94% overlap with a Gaussian) at modest input powers (250 W, peak power or continuous-wave operation). These simulated results reveal two attractive features -- the feasibility of efficiently converting HOMs of fibers into Gaussian-like beams, and the ability to simultaneously perform frequency conversion. Combining the high powers that are possible with HOM fiber amplifiers with access to non-traditional wavelengths may offer significant advantages over the state of the art for many important applications

  17. Harmonics generated from a DC biased transformer

    SciTech Connect

    Shu Lu; Yilu Liu; Ree, J. De La . The Bradley Dept. of Electrical Engineering)

    1993-04-01

    The paper presents harmonic characteristics of transformer excitation currents under DC bias caused by geomagnetically induced currents (GIC). A newly developed saturation model of a single phase shell form transformer based on 3D finite element analysis is used to calculate the excitation currents. As a consequence, the complete variations of excitation current harmonics with respect to an extended range of GIC bias are revealed. The results of this study are useful in understanding transformers as harmonic sources and the impact on power systems during a solar magnetic disturbance.

  18. Efficient millimeter wave 1140 GHz/ diode for harmonic power generation

    NASA Technical Reports Server (NTRS)

    1967-01-01

    Epitaxial gallium arsenide diode junction formed in a crossed waveguide structure operates as a variable reactance harmonic generator. This varactor diode can generate power efficiently in the low-millimeter wavelength.

  19. SEVENTH HARMONIC 20 GHz CO-GENERATOR

    SciTech Connect

    Hirshfield, Jay L

    2014-04-08

    To satisfy the need for multi-MW rf sources in frequency ranges where commercial sources do not exist, a study was undertaken on a class of devices based on gyro-harmonic frequency multiplication. This mechanism relies upon adding energy in gyrating motion to a linear electron beam that traverses a rotating-mode TE111-mode drive cavity in a dc magnetic field. The beam then drifts along the magnetic field into a second cavity, operating in the TEn11-mode tuned to the nth harmonic of the drive cavity. Studies of this configuration have been carried out for 2 < n < 7. Results are given for multi-MW, efficient operation of a 7th harmonic device operating at 20 GHz, and a 2nd harmonic device operating at 22.4 GHz.

  20. High-order harmonic generation in solids: A unifying approach

    NASA Astrophysics Data System (ADS)

    Luu, Tran Trung; Wörner, Hans Jakob

    2016-09-01

    There have been several experimental reports showing high-order harmonic generation from solids, but there has been no unifying theory presented as of yet for all these experiments. Here we report on the systematic investigation of high-order harmonic generation within the semiconductor Bloch equations, taking into account multiple bands and relaxation processes phenomenologically. In addition to reproducing key experiments, we show the following: (i) Electronic excitations, direct-indirect excitation pathways, and relaxation processes are responsible for high-order harmonic generation and control using midinfrared drivers in zinc oxide. We describe an intuitive picture explaining a two-color experiment involving noninversion symmetric crystals. (ii) High-order harmonic generation can be considered as a general feature of ultrafast strong-field-driven electronic dynamics in solids. We demonstrate this statement by predicting high-order harmonic spectra of solids that have not been studied yet.

  1. Illuminating Molecular Symmetries with Bicircular High-Order-Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Reich, Daniel M.; Madsen, Lars Bojer

    2016-09-01

    We present a general theory of bicircular high-order-harmonic generation from N -fold rotationally symmetric molecules. Using a rotating frame of reference we predict the complete structure of the high-order-harmonic spectra for arbitrary driving frequency ratios and show how molecular symmetries can be directly identified from the harmonic signal. Our findings reveal that a characteristic fingerprint of rotational molecular symmetries can be universally observed in the ultrafast response of molecules to strong bicircular fields.

  2. Harmonics Generation by Surface Plasmon Polaritons on Single Nanowires

    PubMed Central

    2016-01-01

    We present experimental observations of visible wavelength second- and third-harmonic generation on single plasmonic nanowires of variable widths. We identify that near-infrared surface plasmon polaritons, which are guided along the nanowire, act as the source of the harmonics generation. We discuss the underlying mechanism of this nonlinear process, using a combination of spatially resolved measurements and numerical simulations to show that the visible harmonics are generated via a combination of both local and propagating plasmonic modes. Our results provide the first demonstration of nanoscale nonlinear optics with guided, propagating plasmonic modes on a lithographically defined chip, opening up new routes toward integrated optical circuits for information processing. PMID:27563688

  3. Spectrum of second-harmonic radiation generated from incoherent light

    SciTech Connect

    Stabinis, A.; Pyragaite, V.; Tamosauskas, G.; Piskarskas, A.

    2011-10-15

    We report on the development of the theory of second-harmonic generation by an incoherent pump with broad angular and frequency spectra. We show that spatial as well as temporal walk-off effects in a nonlinear crystal result in angular dispersion of the second-harmonic radiation. We demonstrate that the acceptance angle in second-harmonic generation by incoherent light is caused by the width of the pump angular spectrum and the resulting angular dispersion of second-harmonic radiation but does not depend on crystal length. In this case the frequency spectrum of second-harmonic radiation is determined by its angular dispersion and the pump angular spectrum. The theory is supported by an experiment in which a LiIO{sub 3} crystal was pumped by a tungsten halogen lamp.

  4. High harmonic generation in a semi-infinite gas cell.

    PubMed

    Sutherland, Julia; Christensen, E; Powers, N; Rhynard, S; Painter, J; Peatross, J

    2004-09-20

    Ten-millijoule 35-femtosecond laser pulses interact with a cell of helium or neon that extends from a focusing lens to an exit foil near the laser focus. High harmonic orders in the range of 50 to 100 are investigated as a function of focal position relative to the exit foil. An aperture placed in front of the focusing lens increases the brightness of observed harmonics by more than an order of magnitude. Counter-propagating light is used to directly probe where the high harmonics are generated within the laser focus. In neon, the harmonics are generated in the last few millimeters before the exit foil, limited by absorption. In helium, the harmonics are produced over a much longer distance. PMID:19483992

  5. Detection of Molecular Monolayers by Optical Second-Harmonic Generation

    SciTech Connect

    Chen, C. K.; Heinz, T. F.; Ricard, D.; Shen, Y. R.

    1980-12-22

    Second harmonic generation is shown to be sensitive enough to detect molecular monolayers adsorbed on a silver surface. Adsorption of AgCl and pyridine on silver during and after an electrolytic cycle can be easily observed,

  6. Frequency-resolved optical grating using third-harmonic generation

    SciTech Connect

    Tsang, T.; Krumbuegel, M.A.; Delong, K.W.

    1995-12-01

    We demonstrate the first frequency-resolved optical gating measurement of an laser oscillator without the time ambiguity using third-harmonic generation. The experiment agrees well with the phase-retrieved spectrograms.

  7. Squeezed light from second-harmonic generation: experiment versus theory.

    PubMed

    Ralph, T C; Taubman, M S; White, A G; McClelland, D E; Bachor, H A

    1995-06-01

    We report excellent quantitative agreement between theoretical predictions and experimental observation of squeezing from a singly resonant second-harmonic-generating crystal. Limitations in the noise suppression imposed by the pump laser are explicitly modeled and confirmed by our measurements.

  8. High order harmonic generation in dual gas multi-jets

    SciTech Connect

    Tosa, Valer E-mail: calin.hojbota@itim-cj.ro; Hojbota, Calin E-mail: calin.hojbota@itim-cj.ro

    2013-11-13

    High order harmonic generation (HHG) in gas media suffers from a low conversion efficiency that has its origins in the interaction of the atom/molecule with the laser field. Phase matching is the main way to enhance the harmonic flux and several solutions have been designed to achieve it. Here we present numerical results modeling HHG in a system of multi-jets in which two gases alternate: the first gas jet (for example Ne) generates harmonics and the second one which ionizes easier, recover the phase matching condition. We obtain configurations which are experimentally feasible with respect to pressures and dimensions of the jets.

  9. Spin-Squeezing Entanglement of Second-Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Shu, Jian

    2016-10-01

    An experimentally feasible scheme for generating spin-squeezing entanglement via second-harmonic generation was presented. Its shown that spin-squeezing entanglement can be generated rapidly in the dynamical process by adjusting coupling constant, detuning, the total number of particles and the evolution time.

  10. Noble gas clusters and nanoplasmas in high harmonic generation

    NASA Astrophysics Data System (ADS)

    Aladi, M.; Bolla, R.; Rácz, P.; Földes, I. B.

    2016-02-01

    We report a study of high harmonic generation from noble gas clusters of xenon atoms in a gas jet. Harmonic spectra were investigated as a function of backing pressure, showing spectral shifts due to the nanoplasma electrons in the clusters. At certain value of laser intensity this process may oppose the effect of the well-known ionization-induced blueshift. In addition, these cluster-induced harmonic redshifts may give the possibility to estimate cluster density and cluster size in the laser-gas jet interaction range.

  11. Control of Laser High-Harmonic Generation with Counterpropagating Light

    NASA Astrophysics Data System (ADS)

    Voronov, S. L.; Kohl, I.; Madsen, J. B.; Simmons, J.; Terry, N.; Titensor, J.; Wang, Q.; Peatross, J.

    2001-09-01

    Relatively weak counterpropagating light is shown to disrupt the emission of laser high-harmonic generation. Harmonic orders ranging from the teens to the low thirties produced by a 30-femtosecond pulse in a narrow argon jet are ``shut down'' with a contrast as high as 2 orders of magnitude by a chirped 1-picosecond counterpropagating laser pulse (60 times less intense). Alternatively, under poor phase-matching conditions, the counterpropagating light boosts harmonic production by similar contrast through quasiphase matching where out-of-phase emission is suppressed.

  12. Quantum theory of third-harmonic generation in graphene

    NASA Astrophysics Data System (ADS)

    Mikhailov, S. A.

    2014-12-01

    A quantum theory of third-harmonic generation in graphene is presented. An analytical formula for the nonlinear conductivity tensor σαβ γ δ (3 )(ω ,ω ,ω ) is derived. Resonant maxima of the third harmonic are shown to exist at low frequencies ω ≪EF/ℏ , as well as around the frequency ω =2 EF/ℏ , where EF is the Fermi energy in graphene. At an input power of a CO2 laser (λ ≈10 μ m ) of about 1 MW /cm2 , the output power of the third harmonic (λ ≈3.3 μ m ) is expected to be ≃50 W /cm2 .

  13. Optical third-harmonic generation using ultrashort laser pulses

    SciTech Connect

    Stoker, D.; Keto, J.W.; Becker, M.F.

    2005-06-15

    To better predict optical third-harmonic generation (THG) in transparent dielectrics, we model a typical ultrashort pulsed Gaussian beam, including both group velocity mismatch and phase mismatch of the fundamental and harmonic fields. We find that competition between the group velocity mismatch and phase mismatch leads to third-harmonic generation that is sensitive only to interfaces. In this case, the spatial resolution is determined by the group velocity walk-off length. THG of modern femtosecond lasers in optical solids is a bulk process, without a surface susceptibility, but bears the signature of a surface enhancement effect in z-scan measurements. We demonstrate the accuracy of the model, by showing the agreement between the predicted spectral intensity and the measured third-harmonic spectrum from a thin sapphire crystal.

  14. Spatiotemporal toroidal waves from the transverse second-harmonic generation.

    PubMed

    Saltiel, Solomon M; Neshev, Dragomir N; Fischer, Robert; Krolikowski, Wieslaw; Arie, Ady; Kivshar, Yuri S

    2008-03-01

    We study the second-harmonic generation via transversely matched interaction of two counterpropagating ultrashort pulses in chi(2) photonic structures. We show that the emitted second-harmonic wave attains the form of spatially expanding toroid with the initial thickness given by the cross correlation of the pulses. We demonstrate the formation of such toroidal waves in crystals with random ferroelectric domains as well as in annularly poled nonlinear photonic structures.

  15. Resonant high-order harmonic generation from plasma ablation: Laser intensity dependence of the harmonic intensity and phase

    SciTech Connect

    Milosevic, D. B.

    2010-02-15

    Experimentally observed strong enhancement of a single high-order harmonic in harmonic generation from low-ionized laser plasma ablation is explained as resonant harmonic generation. The resonant harmonic intensity increases regularly with the increase of the laser intensity, while the phase of the resonant harmonic is almost independent of the laser intensity. This is in sharp contrast with the usual plateau and cutoff harmonics, the intensity of which exhibits wild oscillations while its phase changes rapidly with the laser intensity. The temporal profile of a group of harmonics, which includes the resonant harmonic, has the form of a broad peak in each laser-field half cycle. These characteristics of resonant harmonics can have an important application in attoscience. We illustrate our results using examples of Sn and Sb plasmas.

  16. Generation of higher odd harmonics in a defective photonic crystal

    SciTech Connect

    Ramanujam, N. R.; Wilson, K. S. Joseph

    2015-06-24

    A photonic crystal (AB){sup 2}(DB)(AB){sup 2} with high refractive index medium as silicon and low refractive medium as air is considered. Using the transfer matrix method, the transmission properties as a function of wavelength with photonic band gaps has been obtained. We are able to demonstrate the generation of third, fifth, seventh and ninth harmonics in the present work. We show that if the air medium is removed in the defect, the defect modes are generated but not harmonics. It can be designed to have a frequency conversion, and have a potential for becoming the basis for the next generation of optical devices.

  17. Dynamic investigation of Drosophila myocytes with second harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Greenhalgh, Catherine; Stewart, Bryan; Cisek, Richard; Prent, Nicole; Major, Arkady; Barzda, Virginijus

    2006-09-01

    The functional dynamics and structure of both larval and adult Drosophila melanogaster muscle were investigated with a nonlinear multimodal microscope. Imaging was carried out using a home built microscope capable of recording the multiphoton excitation fluorescence, second harmonic generation, and third harmonic generation signals simultaneously at a scanning rate of up to ~12 frames/sec. The sample was excited by a home built femtosecond Ti:Sapphire laser at 840 nm, or by a Yb-ion doped potassium gadolinium tungstate (Yb:KGW) crystal based oscillator at 1042 nm. There was no observable damage detected in the myocyte after prolonged scanning with either of the lasers. Microscopic second harmonic generation (SHG) appears particularly strong in the myocytes. This allows the fast contraction dynamics of the myocytes to be followed. The larger sarcomere size observed in the larvae myocytes is especially well suited for studying the contraction dynamics. Microscopic imaging of muscle contractions showed different relaxation and contraction rates. The SHG intensities were significantly higher in the relaxed state of the myocyte compared to the contracted state. The imaging also revealed disappearance of SHG signal in highly stretched sarcomeres, indicating that SHG diminishes in the disordered structures. The study illustrates that SHG microscopy, combined with other nonlinear contrast mechanisms, can help to elucidate physiological mechanisms of contraction. This study also provides further insight into the mechanisms of harmonic generation in biological tissue and shows that crystalline arrangement of macromolecules has a determining factor for the high efficiency second harmonic generation from the bulk structures.

  18. Bernstein wave aided laser third harmonic generation in a plasma

    NASA Astrophysics Data System (ADS)

    Tyagi, Yachna; Tripathi, Deepak; Kumar, Ashok

    2016-09-01

    The process of Bernstein wave aided resonant third harmonic generation of laser in a magnetized plasma is investigated. The extra-ordinary mode (X-mode) laser of frequency ω 0 and wave number k → 0 , travelling across the magnetic field in a plasma, exerts a second harmonic ponderomotive force on the electrons imparting them an oscillatory velocity v → 2 ω0 , 2 k → 0 . This velocity beats with the density perturbation due to the Bernstein wave to produce a density perturbation at cyclotron frequency shifted second harmonic. The density perturbation couples with the oscillatory velocity v → ω0 , k → 0 of X-mode of the laser to produce the cyclotron frequency shifted third harmonic current density leading to harmonic radiation. The phase matching condition for the up shifted frequency is satisfied when the Bernstein wave is nearly counter-propagating to the laser. As the transverse wave number of the Bernstein wave is large, it is effective in the phase matched third harmonic generation, when the laser frequency is not too far from the upper hybrid frequency.

  19. Single-shot fluctuations in waveguided high-harmonic generation.

    PubMed

    Goh, S J; Tao, Y; van der Slot, P J M; Bastiaens, H J M; Herek, J; Biedron, S G; Danailov, M B; Milton, S V; Boller, K-J

    2015-09-21

    For exploring the application potential of coherent soft x-ray (SXR) and extreme ultraviolet radiation (XUV) provided by high-harmonic generation, it is important to characterize the central output parameters. Of specific importance are pulse-to-pulse (shot-to-shot) fluctuations of the high-harmonic output energy, fluctuations of the direction of the emission (pointing instabilities), and fluctuations of the beam divergence and shape that reduce the spatial coherence. We present the first single-shot measurements of waveguided high-harmonic generation in a waveguided (capillary-based) geometry. Using a capillary waveguide filled with Argon gas as the nonlinear medium, we provide the first characterization of shot-to-shot fluctuations of the pulse energy, of the divergence and of the beam pointing. We record the strength of these fluctuations vs. two basic input parameters, which are the drive laser pulse energy and the gas pressure in the capillary waveguide. In correlation measurements between single-shot drive laser beam profiles and single-shot high-harmonic beam profiles we prove the absence of drive laser beam-pointing-induced fluctuations in the high-harmonic output. We attribute the main source of high-harmonic fluctuations to ionization-induced nonlinear mode mixing during propagation of the drive laser pulse inside the capillary waveguide. PMID:26406689

  20. Harmonic Generation in Argon by Femtosecond Ti:Sapphire Laser

    NASA Astrophysics Data System (ADS)

    Qindeel, Rabia; Samad, Ricardo Elgul; de Freitas, Anderson Zanardi; de Matos, Paulo Sergio Fabris; Falcão, Edilson Lucena; Vieira Junior, Nilson Dias

    Generation of harmonics using a gas nozzle has remarkable feature in various applications. Pulses from a Ti:Sapphire laser, centered at 785 nm, in a 4 kHz train, with 25 femtoseconds and 800 μJ of maximum energy were employed to generate harmonics in an argon gas nozzle. We present the current results on the focusability of the nozzle, harmonic radiation, measurement of the influence of laser power and laser focus position on the divergence of gas nozzle. We have successfully generated 3rd, 5th and 7th harmonics in Argon at different laser powers. The results show that the harmonic signals are almost same for laser average powers over 1.0 W and variation always appears below 1.0 W. It means that there is saturation in the physical phenomenon happening inside the gas nozzle at high laser powers and the variation is non-linear below 1.0 W. These results are embedded in an effort towards x-ray generation in the water window.

  1. Continuous control of the nonlinearity phase for harmonic generations.

    PubMed

    Li, Guixin; Chen, Shumei; Pholchai, Nitipat; Reineke, Bernhard; Wong, Polis Wing Han; Pun, Edwin Yue Bun; Cheah, Kok Wai; Zentgraf, Thomas; Zhang, Shuang

    2015-06-01

    The capability of locally engineering the nonlinear optical properties of media is crucial in nonlinear optics. Although poling is the most widely employed technique for achieving locally controlled nonlinearity, it leads only to a binary nonlinear state, which is equivalent to a discrete phase change of π in the nonlinear polarizability. Here, inspired by the concept of spin-rotation coupling, we experimentally demonstrate nonlinear metasurfaces with homogeneous linear optical properties but spatially varying effective nonlinear polarizability with continuously controllable phase. The continuous phase control over the local nonlinearity is demonstrated for second and third harmonic generation by using nonlinear metasurfaces consisting of nanoantennas of C3 and C4 rotational symmetries, respectively. The continuous phase engineering of the effective nonlinear polarizability enables complete control over the propagation of harmonic generation signals. Therefore, this method seamlessly combines the generation and manipulation of harmonic waves, paving the way for highly compact nonlinear nanophotonic devices. PMID:25849530

  2. Efficient Forward Second-Harmonic Generation from Planar Archimedean Nanospirals

    DOE PAGES

    Davidson, Roderick B.; Ziegler, Jed I.; Vargas, Guillermo; Avanesyan, Sergey M.; Gong, Yu; Hess, Wayne P.; Haglund, Jr., Richard F.

    2015-05-21

    The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar Archimedean nanospiral offers a unique geometrical asymmetry for second-harmonic generation (SHG) because the SHG results neither from arranging centrosymmetric nanoparticles in asymmetric groupings, nor from noncentrosymmetric nanoparticles that retain a local axis of symmetry. Here we report forward SHG from planar arrays of Archimedean nanospirals using 15 fs pulse from a Ti:sapphire oscillator tuned to 800 nm wavelength. The measured harmonic-generation efficiencies are 2.6•10-9, 8•10-9 and 1.3•10-8 for left-handedmore » circular, linear, and right-handed circular polarizations, respectively.« less

  3. Confocal Imaging of Biological Tissues Using Second Harmonic Generation

    SciTech Connect

    Kim, B-M.; Stoller, P.; Reiser, K.; Eichler, J.; Yan, M.; Rubenchik, A.; Da Silva, L.

    2000-03-06

    A confocal microscopy imaging system was devised to selectively detect Second harmonic signals generated by biological tissues. Several types of biological tissues were examined using this imaging system, including human teeth, bovine blood vessels, and chicken skin. All these tissues generated strong second harmonic signals. There is considerable evidence that the source of these signals in tissue is collagen. Collagen, the predominant component of most tissues, is known to have second order nonlinear susceptibility. This technique may have diagnostic usefulness in pathophysiological conditions characterized by changes in collagen structure including malignant transformation of nevi, progression of diabetic complications, and abnormalities in wound healing.

  4. Optimization study of third harmonic generation in quantum cascade lasers.

    PubMed

    Mojibpour, Ali; Pourfath, Mahdi; Kosina, Hans

    2014-08-25

    A systematic optimization study of quantum cascade lasers with integrated nonlinearity for third-harmonic generation is performed. To model current transport the Pauli master equation is solved using a Monte Carlo approach. A multi-objective particle swarm optimization algorithm is applied to obtain the Pareto front. Our theoretical analysis indicates an optimized structure with five orders of magnitude increase in the generated third-harmonic power with respect to the reference design. This striking performance comes with a low threshold current density of about 1.6 kA/cm2 and is attributed to double resonant phonon scattering assisted extraction and injection scheme of the laser.

  5. Efficient forward second-harmonic generation from planar archimedean nanospirals

    SciTech Connect

    Davidson, II, Roderick B.; Ziegler, Jed I.; Vargas, Guillermo; Avanesyan, Sergey M.; Gong, Yu; Hess, Wayne; Haglund, Jr., Richard F.

    2015-05-01

    Here, the enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar Archimedean nanospiral offers a unique geometrical asymmetry for second-harmonic generation (SHG) because the SHG results neither from arranging centrosymmetric nanoparticles in asymmetric groupings, nor from non-centrosymmetric nanoparticles that retain a local axis of symmetry. Here, we report forward SHG from planar arrays of Archimedean nanospirals using 15 fs pulses from a Ti:sapphire oscillator tuned to 800 nm wavelength.

  6. Even harmonic generation in isotropic media of dissociating homonuclear molecules

    PubMed Central

    Silva, R. E. F.; Rivière, P.; Morales, F.; Smirnova, O.; Ivanov, M.; Martín, F.

    2016-01-01

    Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular gas, only odd harmonics of the driving field can be produced. Here we show how the interplay of electronic and nuclear dynamics can lead to a marked breakdown of this standard picture: a substantial part of the harmonic spectrum can consist of even rather than odd harmonics. We demonstrate the effect using ab-initio solutions of the time-dependent Schrödinger equation for and its isotopes in full dimensionality. By means of a simple analytical model, we identify its physical origin, which is the appearance of a permanent dipole moment in dissociating homonuclear molecules, caused by light-induced localization of the electric charge during dissociation. The effect arises for sufficiently long laser pulses and the region of the spectrum where even harmonics are produced is controlled by pulse duration. Our results (i) show how the interplay of femtosecond nuclear and attosecond electronic dynamics, which affects the charge flow inside the dissociating molecule, is reflected in the nonlinear response, and (ii) force one to augment standard selection rules found in nonlinear optics textbooks by considering light-induced modifications of the medium during the generation process. PMID:27596609

  7. Even harmonic generation in isotropic media of dissociating homonuclear molecules.

    PubMed

    Silva, R E F; Rivière, P; Morales, F; Smirnova, O; Ivanov, M; Martín, F

    2016-01-01

    Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular gas, only odd harmonics of the driving field can be produced. Here we show how the interplay of electronic and nuclear dynamics can lead to a marked breakdown of this standard picture: a substantial part of the harmonic spectrum can consist of even rather than odd harmonics. We demonstrate the effect using ab-initio solutions of the time-dependent Schrödinger equation for and its isotopes in full dimensionality. By means of a simple analytical model, we identify its physical origin, which is the appearance of a permanent dipole moment in dissociating homonuclear molecules, caused by light-induced localization of the electric charge during dissociation. The effect arises for sufficiently long laser pulses and the region of the spectrum where even harmonics are produced is controlled by pulse duration. Our results (i) show how the interplay of femtosecond nuclear and attosecond electronic dynamics, which affects the charge flow inside the dissociating molecule, is reflected in the nonlinear response, and (ii) force one to augment standard selection rules found in nonlinear optics textbooks by considering light-induced modifications of the medium during the generation process. PMID:27596609

  8. Harmonic Generation from Solid Targets - Optmization of Source Parameters

    NASA Astrophysics Data System (ADS)

    Zepf, Matthew; Watts, I. F.; Dangor, A. E.; Norreys, P. A.; Chambers, D. M.; Machacek, A.; Wark, J. S.; Tsakiris, G. D.

    1998-11-01

    High harmonics from solid targets have received renewed interest over the last few years. Theoretical predictions using 1 1/2 D codes suggest that very high orders (>100 ) can be generated at conversion efficiencies in excess of 10-6 [1,2] at Iλ^2 > 10^19 W/cm^2. Experiments have since been performed with pulses varying from 100 fs to 2.5 ps in duration [3-6]. The steep density gradient necessary to generate the harmonics can be generated by either ponderomotive steepening or by using ultraclean pulses which preserve the initial solid vacuum boundary. The two regimes are compared in terms of their dependence on the laser parameters and the emitted harmonic radiation. Particular emphasis will be given to measurements of the holeboring velocity, the polarisation of the harmonics and the intensity scaling in the two regimes. This comparison enables us to find the ideal parameter range for the optimization of harmonic source. [1] R. Lichters et al., Physics of Plasmas 3, 3425, (1996). [2] P. Gibbon, IEEE J. of Q. Elec. 33, 1915 (1997). [3] S. Kohlweyer, et al., Optics Comm. 177, 431 (1995). [4] P. Norreys et al., Phys. Rev. Lett., 76, 1832 (1995). [5] D. von der Linde et al., Phys. Rev. A, 52, R25 (1995) [6] M. Zepf, et al., submitted for publication in Phys. Rev. Lett.

  9. High gain photoconductive semiconductor switching

    SciTech Connect

    Zutavern, F.J.; Loubriel, G.M.; O'Malley, M.W.; Helgeson, W.D.; McLaughlin, D.L.

    1991-01-01

    Switching properties are reported for high gain photoconductive semiconductor switches (PCSS). A 200 ps pulse width laser was used in tests to examine the relations between electric field, rise time, delay, and minimum optical trigger energy for switches which reached 80 kV in a 50 {Omega} transmission line with rise times as short as 600 ps. Infrared photoluminescence was imaged during high gain switching providing direct evidence for current filamentation. Implications of these measurements for the theoretical understanding and practical development of these switches are discussed. 16 refs., 10 figs.

  10. Feasibility study of generating ultra-high harmonic radiation with a single stage echo-enabled harmonic generation scheme

    NASA Astrophysics Data System (ADS)

    Zhou, Kaishang; Feng, Chao; Wang, Dong

    2016-10-01

    The echo enabled harmonic generation (EEHG) scheme holds the ability for the generation of fully coherent soft x-ray free-electron laser (FEL) pulses directly from external UV seeding sources. In this paper, we study the feasibility of using a single stage EEHG to generate coherent radiation in the "water window" and beyond. Using the high-order operating modes of the EEHG scheme, intensive numerical simulations have been performed considering various three-dimensional effects. The simulation results demonstrated that coherent soft x-ray radiation at 150th harmonic (1.77 nm) of the seed can be produced by a single stage EEHG. The decreasing of the final bunching factor at the desired harmonic caused by intra beam scattering (IBS) effect has also been analyzed.

  11. Observation of Electronic Structure Minima in High-Harmonic Generation

    SciTech Connect

    Woerner, Hans Jakob; Villeneuve, D. M.; Niikura, Hiromichi; Bertrand, Julien B.; Corkum, P. B.

    2009-03-13

    We report detailed measurements of the high-harmonic spectra generated from argon atoms. The spectra exhibit a deep minimum that is shown to be independent of the laser intensity, and is thus a clear measure of the electronic structure of the atom. We show that exact field-free continuum wave functions reproduce the minimum, but plane wave and Coulomb wave functions do not. This remarkable observation suggests that electronic structure can be accurately determined in high-harmonic experiments despite the presence of the strong laser field. Our results clarify the relation between high-harmonic generation and photoelectron spectroscopy. The use of exact continuum functions also resolves the ambiguity associated with the choice of the dispersion relation.

  12. Generation of harmonics and supercontinuum in nematic liquid crystals

    SciTech Connect

    Nyushkov, B N; Trashkeev, S I; Klementyev, Vasilii M; Pivtsov, V S; Kobtsev, Sergey M

    2013-02-28

    Nonlinear optical properties of nematic liquid crystals (NLC) have been investigated. A technique for efficient laser frequency conversion in a microscopic NLC volume deposited on an optical fibre end face is experimentally demonstrated. An efficient design of a compact NLC-based IR frequency converter with a fibre input and achromatic collimator is proposed and implemented. Simultaneous generation of the second and third harmonics is obtained for the first time under pumping NLC by a 1.56-mm femtosecond fibre laser. The second-harmonic generation efficiency is measured to be about 1 %, while the efficiency of third-harmonic generation is several tenths of percent. A strong polarisation dependence of the third-harmonic generation efficiency is revealed. When pumping NLC by a cw laser, generation of spectral supercontinua (covering the visible and near-IR spectral ranges) is observed. The nonlinear effects revealed can be due to the light-induced change in the orientational order in liquid crystals, which breaks the initial symmetry and leads to formation of disclination structures. The NLC optical nonlinearity is believed to be of mixed orientationalelectronic nature as a whole. (laser optics 2012)

  13. A microchip laser with intracavity second-harmonic generation

    SciTech Connect

    Derzhavin, S I; Mashkovskii, D A; Timoshkin, V N

    2008-12-31

    A short-pulse 'green' 532-nm Nd{sup 3+}:YVO{sub 4} and KTiOPO{sub 4} microchip laser with intracavity second-harmonic generation, which is pumped by a 809-nm semiconductor laser diode, is developed. (lasers. amplifiers)

  14. Imaging Collagen Orientation Using Polarization-Modulated Second Harmonic Generation

    SciTech Connect

    Stoller, P; Celliers, P M; Reiser, K M; Rubenchik, A M

    2002-01-10

    We use polarization-modulated second harmonic generation to image fiber orientation in collagen tissues, with an axial resolution of about 10 {micro}m and a transverse resolution of up to 1 {micro}m. A linearly polarized ultra-short pulse (200 fs) Ti:Sapphire laser beam is modulated using an electro-optic modulator and quarter-wave plate combination and focused onto a translation stage mounted sample using a microscope objective. The generated second harmonic light is collected using a photomultiplier tube and demodulated using phase sensitive detection to obtain signal intensity and fiber orientation information. In order to obtain second harmonic generation images of different types of collagen organization, we analyze several different tissues, including rat-tail tendon, mouse aorta, mouse fibrotic liver, and porcine skin. We can use our technique to image fibrotic tissue in histological sections of damaged liver and to identify burned tissue in porcine skin to a depth of a few hundred microns. Polarization-modulated second harmonic generation potentially could be a useful clinical technique for diagnosing collagen related disease or damage, especially in the skin.

  15. Modulation compression for short wavelength harmonic generation

    SciTech Connect

    Qiang, J.

    2010-01-11

    Laser modulator is used to seed free electron lasers. In this paper, we propose a scheme to compress the initial laser modulation in the longitudinal phase space by using two opposite sign bunch compressors and two opposite sign energy chirpers. This scheme could potentially reduce the initial modulation wavelength by a factor of C and increase the energy modulation amplitude by a factor of C, where C is the compression factor of the first bunch compressor. Such a compressed energy modulation can be directly used to generate short wavelength current modulation with a large bunching factor.

  16. Classical theory for second-harmonic generation from metallic nanoparticles

    SciTech Connect

    Zeng Yong; Liu Jinjie; Moloney, Jerome V.; Hoyer, Walter; Koch, Stephan W.

    2009-06-15

    In this paper, we develop a classical electrodynamic theory to study the optical nonlinearities of metallic nanoparticles. The quasi free electrons inside the metal are approximated as a classical Coulomb-interacting electron gas, and their motion under the excitation of an external electromagnetic field is described by the plasma equations. This theory is further tailored to study second-harmonic generation. Through detailed experiment-theory comparisons, we validate this classical theory as well as the associated numerical algorithm. It is demonstrated that our theory not only provides qualitative agreement with experiments but it also reproduces the overall strength of the experimentally observed second-harmonic signals.

  17. Effect of Structural Modification on Second Harmonic Generation in Collagen

    SciTech Connect

    Stoller, P C; Reiser, K M; Celliers, P M; Rubenchik, A M

    2003-04-04

    The effects of structural perturbation on second harmonic generation in collagen were investigated. Type I collagen fascicles obtained from rat tails were structurally modified by increasing nonenzymatic cross-linking, by thermal denaturation, by collagenase digestion, or by dehydration. Changes in polarization dependence were observed in the dehydrated samples. Surprisingly, no changes in polarization dependence were observed in highly crosslinked samples, despite significant alterations in packing structure. Complete thermal denaturation and collagenase digestion produced samples with no detectable second harmonic signal. Prior to loss of signal, no change in polarization dependence was observed in partially heated or digested collagen.

  18. Microscopic approach to second harmonic generation in quantum cascade lasers.

    PubMed

    Winge, David O; Lindskog, Martin; Wacker, Andreas

    2014-07-28

    Second harmonic generation is analyzed from a microscopical point of view using a non-equilibrium Green's function formalism. Through this approach the complete on-state of the laser can be modeled and results are compared to experiment with good agreement. In addition, higher order current response is extracted from the calculations and together with waveguide properties, these currents provide the intensity of the second harmonic in the structure considered. This power is compared to experimental results, also with good agreement. Furthermore, our results, which contain all coherences in the system, allow to check the validity of common simplified expressions.

  19. High-order harmonic generation in a capillary discharge

    DOEpatents

    Rocca, Jorge J.; Kapteyn, Henry C.; Mumane, Margaret M.; Gaudiosi, David; Grisham, Michael E.; Popmintchev, Tenio V.; Reagan, Brendan A.

    2010-06-01

    A pre-ionized medium created by a capillary discharge results in more efficient use of laser energy in high-order harmonic generation (HHG) from ions. It extends the cutoff photon energy, and reduces the distortion of the laser pulse as it propagates down the waveguide. The observed enhancements result from a combination of reduced ionization energy loss and reduced ionization-induced defocusing of the driving laser as well as waveguiding of the driving laser pulse. The discharge plasma also provides a means to spectrally tune the harmonics by tailoring the initial level of ionization of the medium.

  20. Tomography of high harmonic generation in a cluster jet.

    PubMed

    Pai, Chih-Hao; Kuo, Cheng-Cheng; Lin, Ming-Wei; Wang, Jyhpyng; Chen, Szu-yuan; Lin, Jiunn-Yuan

    2006-04-01

    Tomographic measurement of high harmonic generation in a cluster jet was demonstrated by programming the cluster density distribution with a laser machining technique. The growth of harmonic energy with the propagation of the pump pulse was resolved by scanning the end of the argon cluster distribution in the path of the pump pulse. A downstream shift of the position of rapid growth and a decrease of the slope with increasing backing pressure as results of changes in the phase-matching condition were observed, which explains the presence of an optimal backing pressure. PMID:16599232

  1. Echo-enabled Harmonic Generation Free Electron Laser

    SciTech Connect

    Xiang, D; Stupakov, G.; /SLAC

    2008-12-18

    In this paper, we systematically study the echo-enabled harmonic generation (EEHG) free electron laser (FEL). The EEHG FEL uses two modulators in combination with two dispersion sections that allow to generate in the beam a high harmonic density modulation starting with a relatively small initial energy modulation of the beam. After presenting analytical theory of the phenomenon, we address several practically important issues, such as the effect of incoherent synchrotron radiation in the dispersion sections, and the beam transverse size effect in the modulator. Using a representative realistic set of beam parameters, we show how the EEHG scheme enhances the FEL performance and allows to generate a fully (both longitudinally and transversely) coherent radiation. As an example, we demonstrate that 5 nm coherent soft x-rays with GW peak power can be generated directly from the 240 nm seeding laser using the proposed EEHG scheme.

  2. Transmit beamforming for optimal second-harmonic generation.

    PubMed

    Hoilund-Kaupang, Halvard; Masoy, Svein-Erik

    2011-08-01

    A simulation study of transmit ultrasound beams from several transducer configurations is conducted to compare second-harmonic imaging at 3.5 MHz and 11 MHz. Second- harmonic generation and the ability to suppress near field echoes are compared. Each transducer configuration is defined by a chosen f-number and focal depth, and the transmit pressure is estimated to not exceed a mechanical index of 1.2. The medium resembles homogeneous muscle tissue with nonlinear elasticity and power-law attenuation. To improve computational efficiency, the KZK equation is utilized, and all transducers are circular-symmetric. Previous literature shows that second-harmonic generation is proportional to the square of the transmit pressure, and that transducer configurations with different transmit frequencies, but equal aperture and focal depth in terms of wavelengths, generate identical second-harmonic fields in terms of shape. Results verify this for a medium with attenuation f1. For attenuation f1.1, deviations are found, and the high frequency subsequently performs worse than the low frequency. The results suggest that high frequencies are less able to suppress near-field echoes in the presence of a heterogeneous body wall than low frequencies.

  3. Evidence of high harmonics from echo-enabled harmonic generation for seeding x-ray free electron lasers.

    PubMed

    Xiang, D; Colby, E; Dunning, M; Gilevich, S; Hast, C; Jobe, K; McCormick, D; Nelson, J; Raubenheimer, T O; Soong, K; Stupakov, G; Szalata, Z; Walz, D; Weathersby, S; Woodley, M

    2012-01-13

    Echo-enabled harmonic generation free electron lasers hold great promise for the generation of fully coherent radiation in x-ray wavelengths. Here we report the first evidence of high harmonics from the echo-enabled harmonic generation technique in the realistic scenario where the laser energy modulation is comparable to the beam slice energy spread. In this experiment, coherent radiation at the seventh harmonic of the second seed laser is generated when the energy modulation amplitude is about 2-3 times the slice energy spread. The experiment confirms the underlying physics of echo-enabled harmonic generation and may have a strong impact on emerging seeded x-ray free electron lasers that are capable of generating laserlike x rays which will advance many areas of science.

  4. Evidence of High Harmonics from Echo-Enabled Harmonic Generation for Seeding X-ray Free Electron Lasers

    SciTech Connect

    Xiang, D.; Colby, E.; Dunning, M.; Gilevich, S.; Hast, C.; Jobe, K.; McCormick, D.; Nelson, J.; Raubenheimer, T.O.; Soong, K.; Stupakov, G.; Szalata, Z.; Walz, D.; Weathersby, S.; Woodle, M.; /SLAC

    2012-02-15

    Echo-enabled harmonic generation free electron lasers hold great promise for the generation of fully coherent radiation in x-ray wavelengths. Here we report the first evidence of high harmonics from the echo-enabled harmonic generation technique in the realistic scenario where the laser energy modulation is comparable to the beam slice energy spread. In this experiment, coherent radiation at the seventh harmonic of the second seed laser is generated when the energy modulation amplitude is about 2-3 times the slice energy spread. The experiment confirms the underlying physics of echo-enabled harmonic generation and may have a strong impact on emerging seeded x-ray free electron lasers that are capable of generating laserlike x rays which will advance many areas of science.

  5. High gain preamplifier based on optical parametric amplification

    DOEpatents

    Jovanovic, Igor; Bonner, Randal A.

    2004-08-10

    A high-gain preamplifier based on optical parametric amplification. A first nonlinear crystal is operatively connected to a second nonlinear crystal. A first beam relay telescope is operatively connected to a second beam relay telescope, to the first nonlinear crystal, and to the second nonlinear crystal. A first harmonic beamsplitter is operatively connected to a second harmonic beamsplitter, to the first nonlinear crystal, to the second nonlinear crystal, to the first beam relay telescope, and to the second beam relay telescope.

  6. Self-Excitation and Harmonics in Wind Power Generation

    SciTech Connect

    Muljadi, E.; Butterfield, C. P.; Romanowitz, H.; Yinger, R.

    2005-11-01

    Traditional wind turbines are commonly equipped with induction generators because they are inexpensive, rugged, and require very little maintenance. Unfortunately, induction generators require reactive power from the grid to operate; capacitor compensation is often used. Because the level of required reactive power varies with the output power, the capacitor compensation must be adjusted as the output power varies. The interactions among the wind turbine, the power network, and the capacitor compensation are important aspects of wind generation that may result in self-excitation and higher harmonic content in the output current. This paper examines the factors that control these phenomena and gives some guidelines on how they can be controlled or eliminated.

  7. Second harmonic generation and enhancement in microfibers and loop resonators

    NASA Astrophysics Data System (ADS)

    Gouveia, Marcelo A.; Lee, Timothy; Ismaeel, Rand; Ding, Ming; Broderick, Neil G. R.; Cordeiro, Cristiano M. B.; Brambilla, Gilberto

    2013-05-01

    We model and experimentally investigate second harmonic generation in silica microfibers and loop resonators, in which the second order nonlinearity arises from the glass-air surface dipole and bulk multipole contributions. In the loop resonator, the recirculation of the pump light on resonance is used to increase the conversion. The effect of the loop parameters, such as coupling and loss, is theoretically studied to determine their influence on the resonance enhancement. Experimentally, microfibers were fabricated with diameters around 0.7 μm to generate the intermodally phase matched second harmonic with an efficiency up to 4.2 × 10-8 when pumped with 5 ns 1.55 μm pulses with a peak power of 90 W. After reconfiguring the microfiber into a 1 mm diameter loop, the efficiency was resonantly enhanced by 5.7 times.

  8. Monitoring microstructural evolution in irradiated steel with second harmonic generation

    NASA Astrophysics Data System (ADS)

    Matlack, Kathryn H.; Kim, Jin-Yeon; Wall, James J.; Qu, Jianmin; Jacobs, Laurence J.

    2015-03-01

    Material damage in structural components is driven by microstructural evolution that occurs at low length scales and begins early in component life. In metals, these microstructural features are known to cause measurable changes in the acoustic nonlinearity parameter. Physically, the interaction of a monochromatic ultrasonic wave with microstructural features such as dislocations, precipitates, and vacancies, generates a second harmonic wave that is proportional to the acoustic nonlinearity parameter. These nonlinear ultrasonic techniques thus have the capability to evaluate initial material damage, particularly before crack initiation and propagation occur. This paper discusses how the nonlinear ultrasonic technique of second harmonic generation can be used as a nondestructive evaluation tool to monitor microstructural changes in steel, focusing on characterizing neutron radiation embrittlement in nuclear reactor pressure vessel steels. Current experimental evidence and analytical models linking microstructural evolution with changes in the acoustic nonlinearity parameter are summarized.

  9. Monitoring microstructural evolution in irradiated steel with second harmonic generation

    SciTech Connect

    Matlack, Kathryn H.; Kim, Jin-Yeon; Jacobs, Laurence J.; Wall, James J.; Qu, Jianmin

    2015-03-31

    Material damage in structural components is driven by microstructural evolution that occurs at low length scales and begins early in component life. In metals, these microstructural features are known to cause measurable changes in the acoustic nonlinearity parameter. Physically, the interaction of a monochromatic ultrasonic wave with microstructural features such as dislocations, precipitates, and vacancies, generates a second harmonic wave that is proportional to the acoustic nonlinearity parameter. These nonlinear ultrasonic techniques thus have the capability to evaluate initial material damage, particularly before crack initiation and propagation occur. This paper discusses how the nonlinear ultrasonic technique of second harmonic generation can be used as a nondestructive evaluation tool to monitor microstructural changes in steel, focusing on characterizing neutron radiation embrittlement in nuclear reactor pressure vessel steels. Current experimental evidence and analytical models linking microstructural evolution with changes in the acoustic nonlinearity parameter are summarized.

  10. Enhanced Harmonic Generation via Breaking of Phase-Matching Symmetry

    NASA Astrophysics Data System (ADS)

    Sergan, Ekaterina; Gibson, George

    2016-05-01

    We discuss experimental results of third harmonic generation (THG) with a focused Gaussian beam in the semi-infinite limit, using two methods. The first method involves placing a metal septum at the waist such that the laser drills a small pinhole, which in turn disrupts the beam after the waist. The second method uses a very thin septum as a separator for two gasses: one with a large third order susceptibility (before the focus), and the other with a small susceptibility (after the focus). Both methods inhibit harmonic generation immediately after the beam waist, leading to increased conversion efficiency and better mode quality. Our work involves studies of conversion efficiency with varying septum thickness and gas pressure, and the results are compared to computer simulations. We would like to acknowledge support from the NSF under Grant No. PHY-1306845.

  11. Continuous third harmonic generation in a terahertz driven modulated nanowire

    NASA Astrophysics Data System (ADS)

    Hamilton, Kathleen E.; Kovalev, Alexey A.; De, Amrit; Pryadko, Leonid P.

    2015-06-01

    We consider the possibility of observing continuous third-harmonic generation using a strongly driven, single-band one-dimensional metal. In the absence of scattering, the quantum efficiency of frequency tripling for such a system can be as high as 93%. Combining the Floquet quasi-energy spectrum with the Keldysh Green's function technique, we derive a semiclassical master equation for a one-dimensional band of strongly and rapidly driven electrons in the presence of weak scattering by phonons. The power absorbed from the driving field is continuously dissipated by phonon modes, leading to a quasi-equilibrium in the electron distribution. We use the Kronig-Penney model with varying effective mass to establish the growth parameters of an InAs/InP nanowire near optimal for third harmonic generation at terahertz frequency range.

  12. Continuous third harmonic generation in a terahertz driven modulated nanowire

    SciTech Connect

    Hamilton, Kathleen E. De, Amrit; Pryadko, Leonid P.; Kovalev, Alexey A.

    2015-06-07

    We consider the possibility of observing continuous third-harmonic generation using a strongly driven, single-band one-dimensional metal. In the absence of scattering, the quantum efficiency of frequency tripling for such a system can be as high as 93%. Combining the Floquet quasi-energy spectrum with the Keldysh Green's function technique, we derive a semiclassical master equation for a one-dimensional band of strongly and rapidly driven electrons in the presence of weak scattering by phonons. The power absorbed from the driving field is continuously dissipated by phonon modes, leading to a quasi-equilibrium in the electron distribution. We use the Kronig-Penney model with varying effective mass to establish the growth parameters of an InAs/InP nanowire near optimal for third harmonic generation at terahertz frequency range.

  13. Corneal imaging by second and third harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Brocas, Arnaud; Jay, Louis; Mottay, Eric; Brunette, Isabelle; Ozaki, Tsuneyuki

    2008-02-01

    Advanced imaging methods are essential tools for improved outcome of refractive surgery. Second harmonic generation (SHG) and third harmonic generation (THG) microscopy are noninvasive high-resolution imaging methods, which can discriminate the different layers of the cornea, thus having strong impact on the outcome of laser surgery. In this work, we use an Ytterbium femtosecond laser as the laser source, the longer wavelength of which reduces scattering, and allows simultaneous SHG and THG imaging. We present SHG and THG images and profiles of pig corneas that clearly show the anterior surface of the cornea, the entry in the stroma and its end, and the posterior surface of the cornea. These observations allow localizing the epithelium, the stroma and the endothelium. Other experiments give information about the structure and cytology of the corneal layers.

  14. Third harmonic generation in exposed-core microstructured optical fibers.

    PubMed

    Warren-Smith, Stephen C; Wie, Jingxuan; Chemnitz, Mario; Kostecki, Roman; Ebendorff-Heidepriem, Heike; Monro, Tanya M; Schmidt, Markus A

    2016-08-01

    Inter-modal phase-matched third harmonic generation has been demonstrated in an exposed-core microstructured optical fiber. Our fiber, with a partially open core having a diameter of just 1.85 µm, shows efficient multi-peak third-harmonic generation between 500 nm and 530 nm, with a maximum visible-wavelength output of 0.96 μW. Mode images and simulations show strong agreement, confirming the phase-matching process and polarization dependence. We anticipate this work will lead to tailorable and tunable visible light sources by exploiting the open access to the optical fiber core, such as depositing thin-film coatings in order to shift the phase matching conditions. PMID:27505753

  15. Vacuum high-harmonic generation in the shock regime

    NASA Astrophysics Data System (ADS)

    Böhl, P.; King, B.; Ruhl, H.

    2015-09-01

    Electrodynamics becomes nonlinear and permits the self-interaction of fields when the quantized nature of vacuum states is taken into account. The effect on a plane probe pulse propagating through a stronger constant crossed background is calculated using numerical simulation and by analytically solving the corresponding wave equation. The electromagnetic shock resulting from vacuum high-harmonic generation is investigated and a nonlinear shock parameter identified.

  16. PHYSICAL BASIS OF QUANTUM ELECTRONICS: Role of a high gain of the medium in superradiance generation and in observation of coherent effects in semiconductor lasers

    NASA Astrophysics Data System (ADS)

    Vasil'ev, Petr P.

    1999-10-01

    A theoretical model of superradiant pulse generation in semiconductor laser structures is developed. It is shown that a high optical gain of the medium can overcome phase relaxation and results in a built-up superradiant state (macroscopic dipole) in an assembly of electron—hole pairs on a time scale much longer than the characteristic polarisation relaxation time T2. A criterion of the superradiance generation is the condition αcmT2>1, where α is the gain coefficient and cm is the speed of light in the medium. The theoretical model describes both qualitatively and quantitatively the author's own experimental results.

  17. High harmonic generation from impulsively aligned SO2

    NASA Astrophysics Data System (ADS)

    Devin, Julien; Wang, Song; Kaldun, Andreas; Bucksbaum, Phil

    2016-05-01

    Previous work in high harmonics generation (HHG) in aligned molecular gases has mainly focused on rotational dynamics in order to determine the contributions of different orbitals to the ionization step. In our experiment, we focus on the shorter timescale of vibrational dynamics. We generate high harmonics from impulsively aligned SO2 molecules in a gas jet and record the emitted attosecond pulse trains in a home-built high resolution vacuum ultra violet (VUV) spectrometer. Using the high temporal resolution of our setup, we are able to map out the effects of vibrational wavepackets with a sub-femtosecond resolution. The target molecule, SO2 gas, is impulsively aligned by a near-infrared laser pulse and has accessible vibrations on the timescale of the short laser pulse used. We present first experimental results for the response to this excitation in high-harmonics. We observe both fast oscillations in the time domain as well as shifts of the VUV photon energy outside of the pulse overlaps. Research supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Chemical Sciences, Geosciences, and Biosciences Division and by the National Science Foundation Graduate Research Fellowship.

  18. Unidirectional high gain brake stop

    NASA Technical Reports Server (NTRS)

    Lang, David J. (Inventor)

    1987-01-01

    This invention relates to a unidirectional high gain brake arrangement that includes in combination a shaft mounted for rotation within a housing. The shaft is rotatable in either direction. A brake is selectively releasably coupled to the housing and to the shaft. The brake has a first member. An intermittent motion device is respectively coupled through the first member to the housing and through a one-way clutch to the shaft. The brake also has a second member that is mechanically coupled to the first brake member and to the housing. The intermittent motion device causes the brake to be activated by movement imparted to the first brake member after a preset number of revolutions of the shaft in one direction. The brake is released by rotation of the shaft in an opposite direction whereby torque transmitted through the one-way clutch to the first brake member is removed.

  19. High-gain antenna & terrain

    NASA Technical Reports Server (NTRS)

    1997-01-01

    Areas of rocky Martian terrain are seen in this image, taken by the Imager for Mars Pathfinder (IMP) on Sol 2. Portions of a lander petal and deflated airbag are at lower left. The dark disk at center is the high-gain antenna, and the silver cylindrical objects at upper right are part of the antenna's mechanism. An area of relatively smooth terrain is seen at upper right, which may offer clues to how this area was formed, and may be a future target for Sojourner's studies. The black area at lower right and small strip at top center is missing data.

    Mars Pathfinder was developed and managed by the Jet Propulsion Laboratory (JPL) for the National Aeronautics and Space Administration. The Imager for Mars Pathfinder (IMP) was developed by the University of Arizona Lunar and Planetary Laboratory under contract to JPL. Peter Smith is the Principal Investigator.

  20. Higher harmonics generation in relativistic electron beam with virtual cathode

    SciTech Connect

    Kurkin, S. A. Badarin, A. A.; Koronovskii, A. A.; Hramov, A. E.

    2014-09-15

    The study of the microwave generation regimes with intense higher harmonics taking place in a high-power vircator consisting of a relativistic electron beam with a virtual cathode has been made. The characteristics of these regimes, in particular, the typical spectra and their variations with the change of the system parameters (beam current, the induction of external magnetic field) as well as physical processes occurring in the system have been analyzed by means of 3D electromagnetic simulation. It has been shown that the system under study demonstrates the tendency to the sufficient growth of the amplitudes of higher harmonics in the spectrum of current oscillations in the VC region with the increase of beam current. The obtained results allow us to consider virtual cathode oscillators as promising high power mmw-to-THz sources.

  1. Higher harmonics generation in relativistic electron beam with virtual cathode

    NASA Astrophysics Data System (ADS)

    Kurkin, S. A.; Badarin, A. A.; Koronovskii, A. A.; Hramov, A. E.

    2014-09-01

    The study of the microwave generation regimes with intense higher harmonics taking place in a high-power vircator consisting of a relativistic electron beam with a virtual cathode has been made. The characteristics of these regimes, in particular, the typical spectra and their variations with the change of the system parameters (beam current, the induction of external magnetic field) as well as physical processes occurring in the system have been analyzed by means of 3D electromagnetic simulation. It has been shown that the system under study demonstrates the tendency to the sufficient growth of the amplitudes of higher harmonics in the spectrum of current oscillations in the VC region with the increase of beam current. The obtained results allow us to consider virtual cathode oscillators as promising high power mmw-to-THz sources.

  2. Electric field induced second harmonic generation with and without fringes

    NASA Astrophysics Data System (ADS)

    Meshulam, G.; Berkovic, G.; Kotler, Z.; Sa'ar, A.

    2000-09-01

    Electric field induced second harmonic generation (EFISH) is a well-known technique to measure the first hyperpolarizability (β) of organic molecules in solution. The characteristic experimental output is observation of oscillatory fringes of second harmonic radiation as the solution path length is changed and evaluation of β from the fringe amplitude. We present two different cases where even in the absence of these characteristic fringes β may still be evaluated: first, when using absorbing materials, and second, when using broadband laser sources. The ability to determine β by EFISH under these conditions greatly enhances the ability of this technique to measure β values over a wide range of laser frequencies. Measurements of the same molecule's β values at different frequencies are reported, verifying the two-level model for the dispersion of β.

  3. Vacuum high-harmonic generation and electromagnetic shock

    NASA Astrophysics Data System (ADS)

    Böhl, P.; King, B.; Ruhl, H.

    2016-04-01

    > When one takes into account the presence of virtual charged states in the quantum vacuum, a nonlinear self-interaction can arise in the propagation of electromagnetic fields. This self-interaction is often referred to as `real photon-photon scattering'. When the centre-of-mass energy of colliding photons is much lower than the rest energy of an electron-positron pair, this quantum effect can be included in the classical field equations of motion as a vacuum current and charge density using the Heisenberg-Euler Lagrangian. Using analytical and numerical methods for subcritical fields, the intrinsic solution to Maxwell's equations has been found for counterpropagating probe and pump plane waves in the presence of vacuum four- and six-wave mixing. In the corresponding all-order solution for the scattered probe, a route to vacuum high-harmonic generation is identified in which a long phase length can compensate for the weakness of interacting fields. The resulting shocks in the probe carrier wave and envelope are studied for different parameter regimes and polarisation set-ups. In this special issue, we study two additional set-ups: that of a slowly varying single-cycle background to highlight the effect of an oscillating background on the probe harmonic spectrum, and that of a few-cycle probe to highlight the smoothing of the harmonic peaks produced by a wider spectrum of probe photons. We also correct sign errors in an earlier publication.

  4. High-harmonic generation from an atomically thin semiconductor

    NASA Astrophysics Data System (ADS)

    Liu, Hanzhe; Li, Yilei; Ghimire, Shambhu; Heinz, Tony; Reis, David

    The process of high-harmonic generation (HHG) from ultrashort laser pulses has recently been observed in bulk solids, complementing the well-established process in the gas phase. HHG is of interest both as a source of ultrashort pulses in the attosecond regime that has photon energies extending up to the soft x-ray region and as a method of probing material response outside the regime of perturbative nonlinear optics. In this paper, we present the observation of HHG from a single atomic layer of MoS2 driven by a strong infrared pulse of 100 fs duration and 0.3 eV photon energy. We observe distinct harmonics up to the 13th order of the infrared excitation. The non-perturbative nature of the HHG process is demonstrated by the weak power dependence of the harmonic intensities. To gain further insight into the process, we have investigated the variation of the HHG signal with sample orientation and the ellipticity of pump excitation. We compare and contrast the process with that from the bulk MoS2 crystal. We find significant differences in the response for the monolayer and bulk crystal, which can be understood in terms of the distinct crystallographic symmetries in the two cases.

  5. High Harmonic Generation from Multiple Orbitals in N2

    SciTech Connect

    McFarland, B.; Farrell, Joseph P.; Bucksbaum, Philip H.; Guehr, Markus; /SLAC, Pulse /Stanford U., Phys. Dept.

    2009-03-05

    Molecular electronic states energetically below the highest occupied molecular orbital (HOMO) should contribute to laser-driven high harmonic generation (HHG), but this behavior has not been observed previously. Our measurements of the HHG spectrum of N{sub 2} molecules aligned perpendicular to the laser polarization showed a maximum at the rotational half-revival. This feature indicates the influence of electrons occupying the orbital just below the N{sub 2} HOMO, referred to as the HOMO-1. Such observations of lower-lying orbitals are essential to understanding subfemtosecond/subangstrom electronic motion in laser-excited molecules.

  6. Second harmonic generation from multilayers of oriented metal bisphosphonates

    SciTech Connect

    Neff, G.A.; Mahon, T.M.; Abshere, T.A.; Page, C.J.

    1996-12-31

    Second order nonlinear optical properties (NLO) require the presence of a polarizable moiety situated in an anharmonic potential. The approach to incorporating such properties into self-assembled multilayers involves use of asymmetric {alpha},{omega} bisphosphonates which meet this requirement by virtue of their chemical structure and binding properties. The authors have developed and optimized protection and deprotection schemes to allow for oriented layering of these molecules. Characterization by optical ellipsometry and grazing angle X-ray diffraction provides insight on average layer thicknesses and bulk film densities. Second harmonic generation (SHG) intensity from the bulk film is measured to verify NLO activity.

  7. Analytic scaling analysis of high harmonic generation conversion efficiency.

    PubMed

    Falcão-Filho, E L; Gkortsas, M; Gordon, Ariel; Kärtner, Franz X

    2009-06-22

    Closed form expressions for the high harmonic generation (HHG) conversion efficiency are obtained for the plateau and cutoff regions. The presented formulas eliminate most of the computational complexity related to HHG simulations, and enable a detailed scaling analysis of HHG efficiency as a function of drive laser parameters and material properties. Moreover, in the total absence of any fitting procedure, the results show excellent agreement with experimental data reported in the literature. Thus, this paper opens new pathways for the global optimization problem of extreme ultraviolet (EUV) sources based on HHG.

  8. Second harmonic generation and crystal growth of substituted thienyl chalcone

    NASA Astrophysics Data System (ADS)

    Goto, Yoshitaka; Hayashi, Akio; Kimura, Yasuhiro; Nakayama, Masaharu

    1991-02-01

    The second harmonic generation (SHG) of 29 kinds of thienyl chalcone derivatives with a thiophene ring were examined. A series of 1-{2-(5-bromothienyl)}-3-(4'-halophenyl)propene-3-one showed high SHG activity. Especially 1-(2-thienyl)-3-(4-methylphenyl)propene-1-one had SHG activity 15 times as large as urea and also high blue light region transparency with a cutoff wavelength of 390 nm. A large high quality single crystal of 60x15x10mm of this compound could be obtained from acetone solution. Analysis of the crystal structure identified it as a monoclinical system of space group P2 1.

  9. Semiclassical analysis of high harmonic generation in bulk crystals

    NASA Astrophysics Data System (ADS)

    Vampa, G.; McDonald, C. R.; Orlando, G.; Corkum, P. B.; Brabec, T.

    2015-02-01

    High harmonic generation (HHG) in solids is investigated. We find that interband emission is dominant for the midinfrared laser driver frequencies, whereas intraband emission dominates the far-infrared range. Interband HHG is similar to atomic HHG and therewith opens the possibility to apply atomic attosecond technology to the condensed matter phase. Interband emission is investigated with a quasiclassical method, by which HHG can be modeled based on the classical trajectory analysis of electron-hole pairs. This analysis yields a simple approximate cutoff law for HHG in solids. Differences between HHG in atoms and solids are identified that are important for adapting atomic attosecond technology to make it applicable to condensed matter.

  10. Correlated Terahertz and High Harmonic Generation from Aligned Nitrogen Molecules

    NASA Astrophysics Data System (ADS)

    Huang, Yindong; Meng, Chao; Wang, Xiaowei; Lv, Zhihui; Zhang, Dongwen; Chen, Wenbo; Zhao, Jing; Yuan, Jianmin; Zhao, Zengxiu

    2016-05-01

    When laser beams are focused on atoms and molecules, wide spectral range of photons can be radiated from the source. In the region of high energy, high harmonic generation (HHG), covering tens to hundreds electron volts, emit within the attosecond timescale. In the low energy region, terahertz wave generation (TWG) can also be generated. Synchronizing TWG with HHG is to take snapshot of the electronic dynamics with time-scale spanning over 6 orders of magnitudes. In this abstract, we report the joint measurements on TWG and HHG from pre-aligned molecules. By calibrating the angular ionization rates with the alignment dependent TWG, we reconstruct the photoionization cross section (PICS) of nitrogen in one run of experiment. The measured PICS is found to be consistent with theoretical predications, although some discrepancies exist. This all-optical method provides a new alternative for investigating molecular structures (Yindong Huang et al., Phys. Rev. Lett. 115, 123002, 2015).

  11. Polarization gating of high harmonic generation in the water window

    NASA Astrophysics Data System (ADS)

    Li, Jie; Ren, Xiaoming; Yin, Yanchun; Cheng, Yan; Cunningham, Eric; Wu, Yi; Chang, Zenghu

    2016-06-01

    We implement the polarization gating (PG) technique with a two-cycle, 1.7 μm driving field to generate an attosecond supercontinuum extending to the water window spectral region. The ellipticity dependence of the high harmonic yield over a photon energy range much broader than previous work is measured and compared with a semi-classical model. When PG is applied, the carrier-envelope phase (CEP) is swept to study its influence on the continuum generation. PG with one-cycle (5.7 fs) and two-cycle (11.3 fs) delay are tested, and both give continuous spectra spanning from 50 to 450 eV under certain CEP values, strongly indicating the generation of isolated attosecond pulses in the water window region.

  12. Designs and numerical calculations for echo-enabled harmonic generation at very high harmonics

    NASA Astrophysics Data System (ADS)

    Penn, G.; Reinsch, M.

    2011-09-01

    The echo-enabled harmonic generation (EEHG) scheme for driving an FEL using two seeded energy modulations at much longer wavelengths than the output wavelength is a promising concept for future seeded FELs. There are many competing requirements in the design of an EEHG beamline which need careful optimization. Furthermore, revised simulation tools and methods are necessary because of both the high harmonic numbers simulated and the complicated nature of the phase space manipulations which are intrinsic to the scheme. This paper explores the constraints on performance and the required tolerances for reaching wavelengths well below 1/100th of that of the seed lasers, and describes some of the methodology for designing such a beamline. Numerical tools, developed both for the GENESIS and GINGER FEL codes, are presented and used here for more accurate study of the scheme beyond a time-averaged model. In particular, the impact of the local structure in peak current and bunching, which is an inherent part of the EEHG scheme, is evaluated.

  13. The effects of harmonics generated by an over-excited transformer on a multimachine system

    SciTech Connect

    Jalali, J.; Mokhtari, S.

    1995-09-01

    An electric power system consisting of three generators and nine buses is considered. The transformer connected to bus seven is considered as a source of harmonics, and it is modeled accordingly. The harmonic source generates harmonics with 6K {+-} 1 orders for K = 1, 2, 3 ..., n. The harmonics of order 6K {+-} 1 with significant effects on different buses of the power system network are evaluated during the steady state operation of the system by using SKM System Software for HIWAVE. Frequency scan and distortion calculations are studied to determine how the harmonics vary the operation of the power system network. The frequency spectrum of the harmonic source indicates that 5th order harmonic affects the operation of the power system. The effects of harmonics on the system are reduced by modeling a single-tuned shunt filter connected to bus seven parallel to the harmonic source to improve the system operation.

  14. Pencil lead plasma for generating multimicrojoule high-order harmonics with a broad spectrum

    SciTech Connect

    Pertot, Y.; Elouga Bom, L. B.; Ozaki, T.; Bhardwaj, V. R.

    2011-03-07

    Using the plasma harmonic method, we show the generation of efficient and intense high-order harmonics from plasma of pencil lead. We demonstrate multimicrojoule energy in each harmonic order for the 11th to the 17th order of a Ti:sapphire laser. By analyzing the target morphology and the plasma composition, we conclude that these intense harmonics are generated from nanoparticles of graphitic carbon.

  15. Diode end pumped laser and harmonic generator using same

    NASA Technical Reports Server (NTRS)

    Byer, Robert L. (Inventor); Dixon, George J. (Inventor); Kane, Thomas J. (Inventor)

    1988-01-01

    A second harmonic, optical generator is disclosed in which a laser diode produces an output pumping beam which is focused by means of a graded, refractive index rod lens into a rod of lasant material, such as Nd:YAG, disposed within an optical resonator to pump the lasant material and to excite the optical resonator at a fundamental wavelength. A non-linear electro-optic material such as MgO:LiNbO.sub.3 is coupled to the excited, fundamental mode of the optical resonator to produce a non-linear interaction with the fundamental wavelength producing a harmonic. In one embodiment, the gain medium and the non-linear material are disposed within an optical resonator defined by a pair of reflectors, one of which is formed on a face of the gain medium and the second of which is formed on a face of the non-linear medium. In another embodiment, the non-linear, electro-optic material is doped with the lasant ion such that the gain medium and the non-linear doubling material are co-extensive in volume. In another embodiment, a non-linear, doubling material is disposed in an optical resonator external of the laser gai medium for improved stability of the second harmonic generation process. In another embodiment, the laser gain medium andthe non-linear material are bonded together by means of an optically transparent cement to form a mechanically stable, monolithic structure. In another embodiment, the non-linear material has reflective faces formed thereon to define a ring resonator to decouple reflections from the non-linear medium back to the gain medium for improved stability.

  16. Enhanced Harmonic Up-Conversion Using a Hybrid HGHG-EEHG Scheme

    SciTech Connect

    Marksteiner, Quinn R.; Bishofberger, Kip A.; Carlsten, Bruce E.; Freund, Henry P.; Yampolsky, Nikolai A.

    2012-04-30

    We introduce a novel harmonic generation scheme which can be used, for a given desired harmonic, to achieve higher bunching factors, weaker chicanes, and/or less final energy spread than can be achieved using Echo-Enabled Harmonic Generation. This scheme only requires a single laser with relatively low power, and is a hybrid of High-Gain Harmonic Generation and EEHG. We present a design of this scheme applied to the Next Generation Light Source (NGLS).

  17. High-harmonic generation in aligned water molecules

    NASA Astrophysics Data System (ADS)

    Wang, Song; Devin, Julien; Hoffmann, Matthias; Cryan, James; Kaldun, Andreas; Bucksbaum, Philip

    2016-05-01

    In recent years, the use of high harmonic generation (HHG) in aligned molecular vapors has become a powerful tool to study ultrafast dynamics of electronic and nuclear wave packets. In our new experimental setup, we are able to orient H2 O and D2 O molecules using a single cycle terahertz (THz) pulse. Aligning water is especially interesting as the highest occupied molecular orbital (HOMO) of water contains a node in the xz plane of the molecular frame, allowing us to perform HHG from second highest occupied molecular orbital (HOMO-1) only, by setting the polarization of the fundamental laser along the z-axis of the aligned water molecules. We are particularly interested in the HOMO-1 state, as there is fast motion of the H-O-H angle leading to sub-wavelength dynamics. On this poster we present our all-optical alignment setup where HHG and single-cycle THz generation take place in high-vacuum, where measurements with arbitrary polarization angles between the two are possible. In addition, we discuss the effects of the molecular orientation on HHG, including symmetry breaking that could produce even harmonics and isotope effects between H2 O and D2 O due to different vibrational energies. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division.

  18. Third Harmonic Generation from Aligned Single-Wall Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Morris, Darius T., Jr.

    Optical properties of single-wall carbon nanotubes (SWCNTs) have been extensively studied during the last decade, and much basic knowledge has been accumulated on how light emission, scattering, and absorption occur in the realm of linear optics. However, their nonlinear optical properties remain largely unexplored. Here, we have observed strong third harmonic generation from highly aligned SWCNTs with intense mid-infrared radiation. Through power dependent experiments, we have determined the absolute value of the third-order nonlinear optical susceptibility, chi(3), of our SWCNT film to be 6.92 x 10--12 esu, which is three orders of magnitude larger than that of the fused silica reference sample we used. Furthermore, through polarization-dependent third harmonic generation experiments, all the nonzero tensor elements of chi(3) have also been extracted. The contribution of the weaker tensor elements to the overall chi (3) signal has been calculated to be approximately 1/6 of that of the dominant c3z zzz component. These results open up new possibilities for application of carbon nanotubes in optoelectronics.

  19. Time-resolved phase-sensitive second harmonic generation spectroscopy.

    PubMed

    Nowakowski, Paweł J; Woods, David A; Bain, Colin D; Verlet, Jan R R

    2015-02-28

    A methodology based on time-resolved, phase-sensitive second harmonic generation (SHG) for probing the excited state dynamics of species at interfaces is presented. It is based on an interference measurement between the SHG from the sample and a local oscillator generated at a reference together with a lock-in measurement to remove the large constant offset from the interference. The technique is characterized by measuring the phase and excited state dynamics of the dye malachite green at the water/air interface. The key attributes of the technique are that the observed signal is directly proportional to sample concentration, in contrast to the quadratic dependence from non-phase sensitive SHG, and that the real and imaginary parts of the 2nd order non-linear susceptibility can be determined independently. We show that the method is highly sensitive and can provide high quality excited state dynamics in short data acquisition times. PMID:25725724

  20. Time-resolved phase-sensitive second harmonic generation spectroscopy

    NASA Astrophysics Data System (ADS)

    Nowakowski, Paweł J.; Woods, David A.; Bain, Colin D.; Verlet, Jan R. R.

    2015-02-01

    A methodology based on time-resolved, phase-sensitive second harmonic generation (SHG) for probing the excited state dynamics of species at interfaces is presented. It is based on an interference measurement between the SHG from the sample and a local oscillator generated at a reference together with a lock-in measurement to remove the large constant offset from the interference. The technique is characterized by measuring the phase and excited state dynamics of the dye malachite green at the water/air interface. The key attributes of the technique are that the observed signal is directly proportional to sample concentration, in contrast to the quadratic dependence from non-phase sensitive SHG, and that the real and imaginary parts of the 2nd order non-linear susceptibility can be determined independently. We show that the method is highly sensitive and can provide high quality excited state dynamics in short data acquisition times.

  1. Resonant second harmonic generation in a gallium nitride two-dimensional photonic crystal on silicon

    NASA Astrophysics Data System (ADS)

    Zeng, Y.; Roland, I.; Checoury, X.; Han, Z.; El Kurdi, M.; Sauvage, S.; Gayral, B.; Brimont, C.; Guillet, T.; Mexis, M.; Semond, F.; Boucaud, P.

    2015-02-01

    We demonstrate second harmonic generation in a gallium nitride photonic crystal cavity embedded in a two-dimensional free-standing photonic crystal platform on silicon. The photonic crystal nanocavity is optically pumped with a continuous-wave laser at telecom wavelengths in the transparency window of the nitride material. The harmonic generation is evidenced by the spectral range of the emitted signal, the quadratic power dependence vs. input power, and the spectral dependence of second harmonic signal. The harmonic emission pattern is correlated to the harmonic polarization generated by the second-order nonlinear susceptibilities χzxx (2 ), χzyy (2 ) and the electric fields of the fundamental cavity mode.

  2. Radially polarized annular beam generated through a second-harmonic-generation process.

    PubMed

    Sato, Shunichi; Kozawa, Yuichi

    2009-10-15

    A radially polarized beam with an annular intensity pattern was generated through a second-harmonic-generation process by focusing an azimuthally polarized Ti:sapphire pulsed laser beam to a c-cut beta-barium borate (BBO) crystal. The annular intensity pattern of the second-harmonic wave had a nearly sixfold symmetry as a result of the nonlinear susceptibility tensor of the BBO crystal. The width of the annulus was as narrow as less than 1/40th of its radius.

  3. Intermyofilament dynamics of myocytes revealed by second harmonic generation microscopy.

    PubMed

    Prent, Nicole; Green, Chantal; Greenhalgh, Catherine; Cisek, Richard; Major, Arkady; Stewart, Bryan; Barzda, Virginijus

    2008-01-01

    Drosophila melanogaster larva myocytes are imaged with second harmonic generation (SHG) microscopy undergoing forced stretching and rhythmic contractions to determine the nature of the SHG signal. During stretching, double peaked SHG profiles of the anisotropic (A-) bands evolve into single peaks with a higher SHG intensity. The dip in the intensity profile at the center of the A-band is attributed to destructive interference from out-of-phase second harmonic radiating myosin molecules that, in the central region of myofilaments, are arranged antiparallel. An intensity increase at the center of the A-band appears during forced stretching due to a small, less than 100 nm, intermyofilament separation of the antiparallel myosin molecules leading to constructive interference of the SHG radiation. In addition, the same phenomenon occurs during periodic contractions of the myocyte, where an SHG intensity increase with the lengthening of sarcomeres is observed. The SHG intensity dependence on sarcomere length can be used for imaging myocyte contractions with low resolution microscopy, and can be applied for the development of diagnostic tools where monitoring of muscle contraction dynamics is required.

  4. Symmetry superposition studied by surface second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Lüpke, G.; Marowsky, G.; Steinhoff, R.; Friedrich, A.; Pettinger, B.; Kolb, D. M.

    1990-04-01

    The components of a third-rank χ(2) tensor have been split into contributions due to 1-fold, 2-fold, 3-fold, and ∞-fold or isotropic rotation axes for a surface of Cs symmetry. Theoretical analysis of the rotation patterns obtained by the surface second-harmonic (SH) generation indicates that a complete symmetry analysis cannot be performed without knowledge of the relevant distribution functions. Rotation axes of lower symmetry create via ``overtones'' or ``harmonics'' contributions apparent in the analysis of the rotation axes of higher symmetry. An experimental example is the observation of structural changes of Au(111) surfaces in an aqueous electrolytic environment. Potential-dependent buildup and removal of a Au(111)-(1×23) surface could be monitored in situ and in real time. Symmetry analysis of the SH rotation patterns reveals both contributions due to a 3-fold axis due to the regular (1×1) structure and simultaneously a 1-fold and a 2-fold axis due to the (1×23) reconstruction.

  5. Harmonic Generation in InAs Nanowire Double Quantum Dots

    NASA Astrophysics Data System (ADS)

    Schroer, M. D.; Jung, M.; Petersson, K. D.; Petta, J. R.

    2012-02-01

    InAs nanowires provide a useful platform for investigating the physics of confined electrons subjected to strong spin-orbit coupling. Using tunable, bottom-gated double quantum dots, we demonstrate electrical driving of single spin resonance.ootnotetextS. Nadj-Perge et al., Nature 468, 1084 (2010)^,ootnotetextM.D. Schroer et al., Phys. Rev. Lett. 107, 176811 (2011) We observe a standard spin response when the applied microwave frequency equals the Larmour frequency f0. However, we also observe an anomalous signal at frequencies fn= f0/ n for integer n up to n ˜5. This is equivalent to generation of harmonics of the spin resonance field. While a f0/2 signal has observed,ootnotetextE.A. Laird et al., Phys. Rev. Lett. 99, 246601 (2007) we believe this is the first observation of higher harmonics in spin resonance. Possible mechanisms will be discussed.ootnotetextE.I. Rashba, arXiv:1110.6569 (2011) Acknowledgements: Research supported by the Sloan and Packard Foundations, the NSF, and Army Research Office.

  6. Resonant second harmonic generation of a Gaussian electromagnetic beam in a collisional magnetoplasma

    SciTech Connect

    Kaur, Sukhdeep; Sharma, A. K.; Salih, Hyder A.

    2009-04-15

    Second harmonic generation of a right circularly polarized Gaussian electromagnetic beam in a magnetized plasma is investigated. The beam causes Ohmic heating of electrons and subsequent redistribution of the plasma, leading to self-defocusing. The radial density gradient, in conjunction with the oscillatory electron velocity, produces density oscillation at the wave frequency. The density oscillation beats with the oscillatory velocity to produce second harmonic current density, giving rise to resonant second harmonic radiation when the wave frequency is one-third of electron cyclotron frequency. The second harmonic field has azimuthal dependence as exp(i{theta}). The self-defocusing causes a reduction in the efficiency of harmonic generation.

  7. Second Harmonic Generation of Nanoscale Phonon Wave Packets

    NASA Astrophysics Data System (ADS)

    Bojahr, A.; Gohlke, M.; Leitenberger, W.; Pudell, J.; Reinhardt, M.; von Reppert, A.; Roessle, M.; Sander, M.; Gaal, P.; Bargheer, M.

    2015-11-01

    Phonons are often regarded as delocalized quasiparticles with certain energy and momentum. The anharmonic interaction of phonons determines macroscopic properties of the solid, such as thermal expansion or thermal conductivity, and a detailed understanding becomes increasingly important for functional nanostructures. Although phonon-phonon scattering processes depicted in simple wave-vector diagrams are the basis of theories describing these macroscopic phenomena, experiments directly accessing these coupling channels are scarce. We synthesize monochromatic acoustic phonon wave packets with only a few cycles to introduce nonlinear phononics as the acoustic counterpart to nonlinear optics. Control of the wave vector, bandwidth, and consequently spatial extent of the phonon wave packets allows us to observe nonlinear phonon interaction, in particular, second harmonic generation, in real time by wave-vector-sensitive Brillouin scattering with x-rays and optical photons.

  8. Second-harmonic generation in zinc tris(thiourea) sulfate

    SciTech Connect

    Marcy, H.O.; Warren, L.F. ); Webb, M.S.; Ebbers, C.A.; Velsko, S.P. ); Kennedy, G.C.; Catella, G.C. )

    1992-08-20

    The linear and second-order nonlinear optical properties of single-crystal zinc tris(thiourea) sulfate, or ZTS, are determined. The deduced nonlinear coefficients are {vert bar} {ital d}{sub 31} {vert bar}=0.31, {vert bar} {ital d}{sub 32} {vert bar}=0.35, and {vert bar} {ital d}{sub 33} {vert bar}=0.23 pm/V compared with a {vert bar} {ital d}{sub 14} {vert bar} value of 0.39 pm/V for potassium dihydrogen phosphate. Because it exhibits a low angular sensitivity ({delta}{Delta}{ital k}/{delta}{theta}), ZTS may prove useful for type-II second-harmonic generation from 1.06 to 1.027 {mu}m. We present the phase-matching measurement data for ZTS and compare the calculated frequency conversion efficiency for ZTS with that of several other well-characterized materials.

  9. High harmonic generation in the undulators for free electron lasers

    NASA Astrophysics Data System (ADS)

    Zhukovsky, K.

    2015-10-01

    We present the analysis of the undulator radiation (UR) with account for major sources of the spectral line broadening. For relativistic electrons we obtain the analytical expressions for the UR spectrum, the intensity and the emission line shape with account for the finite size of the beam, the emittance and the energy spread. Partial compensation of the divergency by properly imposed weak constant magnetic component is demonstrated in the analytical form. Considering the examples of radiation from single and double frequency undulators, we study high harmonic generation with account for all major sources of homogeneous and inhomogeneous broadening with account for the characteristics of the electrons beam. We apply our analysis to free electron laser (FEL) calculations and we compare the obtained results with the radiation of a FEL on the supposition of the ideal undulator.

  10. On probing conformation of microtubules by second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Sharoukhov, Denis; Lim, Hyungsik

    2016-01-01

    Microtubule (MT) is a component of cytoskeleton playing an important role in a variety of cellular processes. Altering the structure of MT is a crucial mechanism of modulating the function, but it is difficult to measure the in vivo conformation. We present here the use of second-harmonic generation (SHG) for acquiring information about the architecture of MTs in living tissue. Axonal MTs were imaged by polarization-resolved SHG and anisotropy in the molecular structure was determined by means of the second-order tensor analysis. The feasibility of the second-order tensor analysis was tested for measuring the conformational changes induced by MT-stabilizing drug. It demonstrates that the new optical contrast may be useful for investigating the dynamics of MT cytoskeleton in vivo.

  11. Interpreting Second-Harmonic Generation Images of Collagen I Fibrils

    PubMed Central

    Williams, Rebecca M.; Zipfel, Warren R.; Webb, Watt W.

    2005-01-01

    Fibrillar collagen, being highly noncentrosymmetric, possesses a tremendous nonlinear susceptibility. As a result, second-harmonic generation (SHG) microscopy of collagen produces extremely bright and robust signals, providing an invaluable tool for imaging tissue structure with submicron resolution. Here we discuss fundamental principles governing SHG phase matching with the tightly focusing optics used in microscopy. Their application to collagen imaging yields several biophysical features characteristic of native collagen structure: SHG radiates from the shell of a collagen fibril, rather than from its bulk. This SHG shell may correspond to the supporting element of the fibril. Physiologically relevant changes in solution ionic strength alter the ratio of forward-to-backward propagating SHG, implying a resulting change in the SHG shell thickness. Fibrillogenesis can be resolved in immature tissue by directly imaging backward-propagating SHG. Such findings are crucial to the design and development of forthcoming diagnostic and research tools. PMID:15533922

  12. Second Harmonic Generation in a Graphe Armchair Nanoribbon

    NASA Astrophysics Data System (ADS)

    Gumbs, Godfrey; Abranyos, Yonatan

    2013-03-01

    The second order nonlinear optical susceptibility χ (2) for second harmonic generation is calculated for the 11H transition of a graded double quantum well (DQW) structure of undoped- GaAs / Alx Ga1 - x As . These results are compared with the single quantum well (QW). Our results show that the values of χ (2) have optimal magnitudes dependent on the width, depth and separation between the QWs in a DQW structure. When the electric field increases, the dipole moment increases due to the increasing separation between the electron and hole wave functions. On the other hand, the oscillator strength of the 11H transition is reduced as a result of the decrease in the overlap of the electron and hole envelope functions. These two competing factors give rise to optimal conditions for the enhancement of the second order nonlinear susceptibility χ (2). It is demonstrated that χ (2) for the DQW structure is more enhanced than for the biased single QW.

  13. High-order harmonic generation enhanced by XUV light

    SciTech Connect

    Buth, Christian; Kohler, Markus C.; Ullrich, Joachim; Keitel, Christoph H.

    2012-03-19

    The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the first electron performs a HHG three-step process, whereas the second electron Rabi flops between the core and the valence vacancy. The modified HHG spectrum due to recombination with the valence and the core is determined and analyzed for krypton on the 3d {yields} 4p resonance in the ion. We assume an 800 nm laser with an intensity of about 10{sup 14} Wcm{sup 2} and XUV radiation from the Free Electron Laser in Hamburg (FLASH) with an intensity in the range 10{sup 13}-10{sup 16} Wcm{sup 2}. Our prediction opens perspectives for nonlinear XUV physics, attosecond x rays, and HHG-based spectroscopy involving core orbitals.

  14. Second harmonic generation and crystal growth of new chalcone derivatives

    NASA Astrophysics Data System (ADS)

    Patil, P. S.; Dharmaprakash, S. M.; Ramakrishna, K.; Fun, Hoong-Kun; Sai Santosh Kumar, R.; Narayana Rao, D.

    2007-05-01

    We report on the synthesis, crystal structure and optical characterization of chalcone derivatives developed for second-order nonlinear optics. The investigation of a series of five chalcone derivatives with the second harmonic generation powder test according to Kurtz and Perry revealed that these chalcones show efficient second-order nonlinear activity. Among them, high-quality single crystals of 3-Br-4'-methoxychalcone (3BMC) were grown by solvent evaporation solution growth technique. Grown crystals were characterized by X-ray powder diffraction (XRD), laser damage threshold, UV-vis-NIR and refractive index measurement studies. Infrared spectroscopy, thermogravimetric analysis and differential thermal analysis measurements were performed to study the molecular vibration and thermal behavior of 3BMC crystal. Thermal analysis does not show any structural phase transition.

  15. Electromagnetic study of second harmonic generation by a corrugated waveguide

    NASA Astrophysics Data System (ADS)

    Neviere, Michel; Popov, E.; Reinisch, Raymond

    1995-09-01

    When an incident plane wave with circular frequency (omega) falls on a grating coated by a layer of nonlinear material, it generates a nonlinear polarization PNL(2(omega) ) which acts as a source term and produces a second harmonic (SH) field called signal. The excitation of an electromagnetic resonance like surface plasmon or a guided wave increases the local field and thus the signal. The problem is to be able to compute and optimize the latter. We have developed a new theory which uses a coordinate transformation mapping the grating profile onto a plane. This simplifies the boundary conditions but complicates the propagation equation. Taking advantage of the psuedoperiodicity of the problem, the Fourier harmonics of the field are solution of a set of first order differential equations with constant coefficients. The resolution of this system via eigenvalue and eigenvector technique avoid numerical instabilities and lead to accurate results which agree perfectly with those found via the Rayleigh method or by the Differential method, when they work. A phenomenological approach is then developed to explain the unusual shape of the resonance lines at 2(omega) , which is based on the poles and zeros of the scattering operator S at (omega) and 2(omega) . It is shown that S(2(omega) ) presents 3 complex poles with 3 associated complex zeros. Their knowledge, plus the nonlinear reflectivity of the plane device allows predicting all the possible shapes of the 2(omega) signal as a function of angle of incidence. The phenomenological study explains an experimental result, found a few years ago, that if 2(omega) lies inside the absorption band of the guiding material instead of the transparent region, the enhanced second harmonic generation (SHG) is changed into a reduced one. It means that in the case phase matching can lead to a minimum instead of maximum. An algorithm is then proposed to maximize the signal intensity; with polyurethane as a guiding material a conversion

  16. Polarization-Modulated Second Harmonic Generation Microscopy in Collagen

    SciTech Connect

    Stoller, P C

    2002-09-30

    Collagen is a key structural protein in the body; several pathological conditions lead to changes in collagen. Among imaging modalities that can be used in vivo, second harmonic generation (SHG) microscopy has a key advantage: it provides {approx}1 {micro}m resolution information about collagen structure as a function of depth. A new technique--polarization-modulated SHG--is presented: it permits simultaneous measurement of collagen orientation, of a lower bound on the magnitude of the second order nonlinear susceptibility tensor, and of the ratio of the two independent elements in this tensor. It is applied to characterizing SHG in collagen and to determining effects of biologically relevant changes in collagen structure. The magnitude of the second harmonic signal in two dimensional images varies with position even in structurally homogeneous tissue; this phenomenon is due to interference between second harmonic light generated by neighboring fibrils, which are randomly oriented parallel or anti-parallel to each other. Studies in which focal spot size was varied indicated that regions where fibrils are co-oriented are less than {approx}1.5 {micro}m in diameter. A quartz reference was used to determine the spot size as well as a lower limit (d{sub xxx} > 0.3 pm/V) for the magnitude of the second order nonlinear susceptibility. The ratio of the two independent tensor elements ranged between d{sub XYY}/d{sub XXX} = 0.60 and 0.75. SHG magnitude alone was not useful for identifying structural anomalies in collagenous tissue. Instead, changes in the polarization dependence of SHG were used to analyze biologically relevant perturbations in collagen structure. Changes in polarization dependence were observed in dehydrated samples, but not in highly crosslinked samples, despite significant alterations in packing structure. Complete thermal denaturation and collagenase digestion produced samples with no detectable SHG signal. Collagen orientation was measured in thin

  17. Recent Progress in High-Gain FEL Theory

    SciTech Connect

    Huang, Z.; /SLAC

    2005-09-30

    High-gain free electron lasers (FEL) are being developed as extremely bright x-ray sources of a next-generation radiation facility. In this paper, we review the basic theory and the recent progress in understanding the startup, the exponential growth and the saturation of the high-gain process, emphasizing the self-amplified spontaneous emission (SASE). We will also discuss how the FEL performance may be affected by various errors and wakefield effects in the undulator.

  18. Optical Cherenkov radiation in ultrafast cascaded second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Bache, M.; Bang, O.; Zhou, B. B.; Moses, J.; Wise, F. W.

    2010-12-01

    We show through theory and numerics that when few-cycle femtosecond solitons are generated through cascaded (phase-mismatched) second-harmonic generation, these broadband solitons can emit optical Cherenkov radiation in the form of linear dispersive waves located in the red part of the spectrum. The beating between the dispersive wave and the soliton generates trailing temporal oscillations on the compressed soliton. Insertion of a simple short-wave pass filter after the crystal can restore a clean soliton. On the other hand, bandpass filtering around the dispersive wave peak results in near-transform-limited ultrashort mid-IR pulses with pulse durations much shorter than the input near-IR pulse. The Cherenkov radiation for the crystal considered (β-barium borate) is found for pump wavelengths in the range λ=0.95-1.45μm, and is located in the regime λ=1.5-3.5μm. For shorter pump wavelengths, the phase-matching point is located in the absorption region of the crystal, effectively absorbing the generated dispersive wave. By calculating the phase-matching curves for typically used frequency conversion crystals, we point out that the mid-IR absorption in the crystal in many cases automatically will filter away the dispersive wave. Finally, an investigation of recent experimental results uncovers a four-wave-mixing phenomenon related to Cherenkov radiation that is an additional generation mechanism of long-wavelength radiation that can occur during soliton compression. We discuss the conditions that lead to this alternative dynamics rather than generation of Cherenkov radiation.

  19. Second harmonic generation from an individual amorphous selenium nanosphere

    NASA Astrophysics Data System (ADS)

    Ma, C. R.; Yan, J. H.; Wei, Y. M.; Yang, G. W.

    2016-10-01

    Among the numerous nonlinear optics effects, second harmonic generation (SHG) is always a hotspot and it is extensively used for optical frequency conversion, biomedical imaging, etc. However, SHG is forbidden in a medium with inversion symmetry under the electric-dipole approximation. Here, we demonstrated SHG from a single amorphous selenium (a-Se) nanosphere under near-infrared femtosecond pulse excitation. It was found that SH spectra are tunable with the size of a-Se nanospheres and the SHG efficiency of a single a-Se sphere with a diameter over 300 nm is estimated at 10-8. We also established two physical mechanisms of SHG from the amorphous nanospheres. There is an electric-dipole contribution to the second-order nonlinearity in view of the inevitable structural discontinuity at the surface. The discontinuity of the normal component of the electric field strength leads to the quadrupole-type contributions arising from the large electric field gradient. The SHG process can be enhanced by resonance near the fundamental wavelength, giving rise to the detectable second harmonic (SH) spectra of a single a-Se nanosphere (d > 300 nm) or two small a-Se nanospheres (d = 200 nm) aggregated into a dimer, while the single nanosphere with smaller size (d > 300 nm) is undetectable. As an essential trace element for animals, a-Se features unique biological compatibility and has specific properties of optical nonlinearity within the optical window in biological tissue. This discovery makes a-Se nanospheres promising both in nonlinear optics and biomedicine.

  20. Second harmonic generation from an individual amorphous selenium nanosphere.

    PubMed

    Ma, C R; Yan, J H; Wei, Y M; Yang, G W

    2016-10-21

    Among the numerous nonlinear optics effects, second harmonic generation (SHG) is always a hotspot and it is extensively used for optical frequency conversion, biomedical imaging, etc. However, SHG is forbidden in a medium with inversion symmetry under the electric-dipole approximation. Here, we demonstrated SHG from a single amorphous selenium (a-Se) nanosphere under near-infrared femtosecond pulse excitation. It was found that SH spectra are tunable with the size of a-Se nanospheres and the SHG efficiency of a single a-Se sphere with a diameter over 300 nm is estimated at 10(-8). We also established two physical mechanisms of SHG from the amorphous nanospheres. There is an electric-dipole contribution to the second-order nonlinearity in view of the inevitable structural discontinuity at the surface. The discontinuity of the normal component of the electric field strength leads to the quadrupole-type contributions arising from the large electric field gradient. The SHG process can be enhanced by resonance near the fundamental wavelength, giving rise to the detectable second harmonic (SH) spectra of a single a-Se nanosphere (d > 300 nm) or two small a-Se nanospheres (d = 200 nm) aggregated into a dimer, while the single nanosphere with smaller size (d > 300 nm) is undetectable. As an essential trace element for animals, a-Se features unique biological compatibility and has specific properties of optical nonlinearity within the optical window in biological tissue. This discovery makes a-Se nanospheres promising both in nonlinear optics and biomedicine. PMID:27632529

  1. Second harmonic generation from an individual amorphous selenium nanosphere.

    PubMed

    Ma, C R; Yan, J H; Wei, Y M; Yang, G W

    2016-10-21

    Among the numerous nonlinear optics effects, second harmonic generation (SHG) is always a hotspot and it is extensively used for optical frequency conversion, biomedical imaging, etc. However, SHG is forbidden in a medium with inversion symmetry under the electric-dipole approximation. Here, we demonstrated SHG from a single amorphous selenium (a-Se) nanosphere under near-infrared femtosecond pulse excitation. It was found that SH spectra are tunable with the size of a-Se nanospheres and the SHG efficiency of a single a-Se sphere with a diameter over 300 nm is estimated at 10(-8). We also established two physical mechanisms of SHG from the amorphous nanospheres. There is an electric-dipole contribution to the second-order nonlinearity in view of the inevitable structural discontinuity at the surface. The discontinuity of the normal component of the electric field strength leads to the quadrupole-type contributions arising from the large electric field gradient. The SHG process can be enhanced by resonance near the fundamental wavelength, giving rise to the detectable second harmonic (SH) spectra of a single a-Se nanosphere (d > 300 nm) or two small a-Se nanospheres (d = 200 nm) aggregated into a dimer, while the single nanosphere with smaller size (d > 300 nm) is undetectable. As an essential trace element for animals, a-Se features unique biological compatibility and has specific properties of optical nonlinearity within the optical window in biological tissue. This discovery makes a-Se nanospheres promising both in nonlinear optics and biomedicine.

  2. Numerical studies of third-harmonic generation in laser filament in air perturbed by plasma spot

    SciTech Connect

    Feng Liubin; Lu Xin; Liu Xiaolong; Li Yutong; Chen Liming; Ma Jinglong; Dong Quanli; Wang Weimin; Xi Tingting; Sheng Zhengming; Zhang Jie; He Duanwei

    2012-07-15

    Third-harmonic emission from laser filament intercepted by plasma spot is studied by numerical simulations. Significant enhancement of the third-harmonic generation is obtained due to the disturbance of the additional plasma. The contribution of the pure plasma effect and the possible plasma-enhanced third-order susceptibility on the third-harmonic generation enhancement are compared. It is shown that the plasma induced cancellation of destructive interference [Y. Liu et al., Opt. Commun. 284, 4706 (2011)] of two-colored filament is the dominant mechanism of the enhancement of third-harmonic generation.

  3. Avalanche of stimulated forward scattering in high harmonic generation.

    PubMed

    Serrat, Carles; Roca, David; Budesca, Josep M; Seres, Jozsef; Seres, Enikoe; Aurand, Bastian; Hoffmann, Andreas; Namba, Shinichi; Kuehl, Thomas; Spielmann, Christian

    2016-04-18

    Optical amplifiers in all ranges of the electromagnetic spectrum exhibit an essential characteristic, namely the input signal during the propagation in the amplifier medium is multiplied by the avalanche effect of the stimulated emission to produce exponential growth. We perform a theoretical study motivated and supported by experimental data on a He gas amplifier driven by intense 30-fs-long laser pulses and seeded with attosecond pulse trains generated in a separated Ne gas jet. We demonstrate that the strong-field theory in the frame of high harmonic generation fully supports the appearance of the avalanche effect in the amplification of extreme ultraviolet attosecond pulse trains. We theoretically separate and identify different physical processes taking part in the interaction and we demonstrate that X-ray parametric amplification dominates over others. In particular, we identify strong-field mediated intrapulse X-ray parametric processes as decisive for amplification at the single-atom level. We confirm that the amplification takes place at photon energies where the amplifier is seeded and when the seed pulses are perfectly synchronized with the driving strong field in the amplifier. Furthermore, propagation effects, phase matching and seed synchronization can be exploited to tune the amplified spectral range within the seed bandwidth. PMID:27137242

  4. Third harmonic generation microscopy of a mouse retina

    PubMed Central

    Lei, Tim C.; Domingue, Scott R.; Kahook, Malik Y.; Bartels, Randy A.; Ammar, David A.

    2015-01-01

    Purpose To demonstrate lipid-specific imaging of the retina through the use of third harmonic generation (THG), a multiphoton microscopic technique in which tissue contrast is generated from optical inhomogeneities. Methods A custom fiber laser and multiphoton microscope was constructed and optimized for simultaneous two-photon autofluorescence (TPAF) and THG retinal imaging. Imaging was performed using fixed-frozen sections of mouse eyes without the use of exogenous fluorescent dyes. In parallel experiments, a fluorescent nuclear stain was used to verify the location of the retinal cell nuclei. Results Simultaneous THG and TPAF images revealed all retinal layers with subcellular resolution. In BALB/c strains, the THG signal stems from the lipidic organelles of the cellular and nuclear membranes. In the C57BL/6 strain, the THG signal from the RPE cells originates from the pigmented granules. Conclusions THG microscopy can be used to image structures of the mouse retina using contrast inherent to the tissue and without the use of a fluorescent dye or exogenously expressed recombinant protein. PMID:25999681

  5. High-order harmonic generation directly from a filament

    NASA Astrophysics Data System (ADS)

    Steingrube, D. S.; Schulz, E.; Binhammer, T.; Gaarde, M. B.; Couairon, A.; Morgner, U.; Kovačev, M.

    2011-04-01

    The synthesis of isolated attosecond pulses (IAPs) in the extreme ultraviolet (XUV) spectral region has opened up the shortest time scales for time-resolved studies. It relies on the generation of high-order harmonics (HHG) from high-power few-cycle infrared (IR) laser pulses. Here we explore experimentally a new and simple route to IAP generation directly from 35 fs IR pulses that undergo filamentation in argon. Spectral broadening, self-shortening of the IR pulse and HHG are realized in a single stage, reducing the cost and experimental effort for easier spreading of attosecond sources. We observe continuous XUV spectra supporting IAPs, emerging directly from the filament via a truncating pinhole to vacuum. The extremely short absorption length of the XUV radiation makes it a highly local probe for studying the elusive filamentation dynamics and in particular provides an experimental diagnostic of short-lived spikes in laser intensity. The excellent agreement with numerical simulations suggests the formation of a single-cycle pulse in the filament.

  6. Imaging leukocytes in vivo with third harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Tsai, Cheng-Kun; Chen, Chien-Kuo; Chen, Yu-Shing; Wu, Pei-Chun; Hsieh, Tsung-Yuan; Liu, Han-Wen; Yeh, Chiou-Yueh; Lin, Win-Li; Chia, Jean-San; Liu, Tzu-Ming

    2013-02-01

    Without a labeling, we demonstrated that lipid granules in leukocytes have distinctive third harmonic generation (THG) contrast. Excited by a 1230nm femtosecond laser, THG signals were generated at a significantly higher level in neutrophils than other mononuclear cells, whereas signals in agranular lymphocytes were one order smaller. These characteristic THG features can also be observed in vivo to trace the newly recruited leukocytes following lipopolysaccharide (LPS) challenge. Furthermore, using video-rate THG microscopy, we also captured images of blood cells in human capillaries. Quite different from red-blood-cells, every now and then, round and granule rich blood cells with strong THG contrast appeared in circulation. The corresponding volume densities in blood, evaluated from their frequencies of appearance and the velocity of circulation, fall within the physiological range of human white blood cell counts. These results suggested that labeling-free THG imaging may provide timely tracing of leukocyte movement and hematology inspection without disturbing the normal cellular or physiological status.

  7. Angularly separated harmonic generation from intense laser interaction with blazed diffraction gratings.

    PubMed

    Yeung, M; Zepf, M; Geissler, M; Dromey, B

    2011-06-15

    We made numerical simulations of the generation of narrowband beams of extreme ultraviolet radiation from intense laser interaction with a blazed grating surface. Strong fifth harmonic emission into its blazed diffraction order was observed as well as heavy suppression of the fundamental frequency with comparison to a typical harmonic spectrum from a flat target. The results demonstrate a new highly efficient method of generating near-monochromatic harmonics from the fundamental with minimal effect on the pulse duration.

  8. Application of organic compounds for high-order harmonic generation of ultrashort pulses

    NASA Astrophysics Data System (ADS)

    Ganeev, R. A.

    2016-02-01

    The studies of the high-order nonlinear optical properties of a few organic compounds (polyvinyl alcohol, polyethylene, sugar, coffee, and leaf) are reported. Harmonic generation in the laser-produced plasmas containing the molecules and large particles of above materials is demonstrated. These studies showed that the harmonic distributions and harmonic cutoffs from organic compound plasmas were similar to those from the graphite ablation. The characteristic feature of observed harmonic spectra was the presence of bluesided lobes near the lower-order harmonics.

  9. High-order harmonic generation from C{sub 60}-rich plasma

    SciTech Connect

    Ganeev, R. A.; Elouga Bom, L. B.; Ozaki, T.; Wong, M. C. H.; Brichta, J.-P.; Bhardwaj, V. R.; Redkin, P. V.

    2009-10-15

    We performed systematic investigation of high-order harmonic generation from fullerene-rich laser-produced plasmas. We studied harmonic generation by varying several experimental parameters, such as the delay between the ablation and driving pulses, and divergence and polarization of the pump laser. Enhancement of harmonic yield is observed near 20 eV, which is attributed to the influence of a broadband plasmon resonance of C{sub 60} on the nonlinear optical response of fullerene-rich plasma. This increase in the harmonic intensity occurs despite the increased absorption by C{sub 60} at these wavelengths. Using simulations based on time-dependent density-functional theory, we confirm that this effect is due to the influence of collective excitations. We compare harmonic generation from fullerenes using lasers with 793 nm and 396 nm wavelengths, which show the influence of plasmon resonance on the conversion efficiency of high-order harmonics for different laser wavelengths.

  10. Contribution of longitudinal electric field of a gaussian beam to second harmonic generation

    NASA Astrophysics Data System (ADS)

    Mishra, S. R.; Rustagi, K. C.

    1990-01-01

    A laser beam with a nonuniform transverse intensity profile necessarily has a longitudinal component of the electric field. We show that a detectable second harmonic can be generated due to coupling of this longitudinal component with the transverse field of a gaussian beam in a configuration in which second harmonic generation is forbidden for plane wave interaction.

  11. Predicting bulk damage in NIF triple harmonic generators

    SciTech Connect

    De Yoreo, J; Runkel, M; Williams, W

    1998-09-18

    Recently reported experiments have investigated the statistics of laser damage in KDP and KD*P. Automated damage tests have allowed cumulative failure and damage probability distributions to be constructed. Large area tests have investigated the feasibility of on-line laser conditioning and damage evolution for tripler harmonic generation (THG) crystals on the National Ignition Facility (NIF). These tests have shown that there is a nonzero probability of damage at NIF redline fluence (14.3 J/cm2, 351 nm, 3 ns) and that the damage pinpoint density evolves exponentially with fluence. In this paper, the results of these tests are used in conjunction with model spatial profiles of the NIP beam to predict the level of damage created in the THG crystal. A probabilistic calculation based on the overlap of the beam fluence and damage probabiity distribution shows that the overall damage probability is less than 3% for well-conditioned, high quality KDP/KD*P crystals of conventional or rapid growth. The number density of generated pinpoints has been calculated by mapping the damage evolution curves onto the NlF model profile. This shows that the number of damage pinpoints generated in high fluence portions of the NIF beam will be low for well-conditioned THG crystals. In contrast, unconditioned triplers of the same material will exhibit an increase in pinpoint density of greater than 20x. To test the validity of these calculations a 37 cm, conventionally grown KD*P tripler from the Beamlet laser was scatter mapped for bulk damage. The tripler had been exposed to NE-like fluences during its operational lifetime on Beamlet and exhibited very low levels of bulk pinpoint damage, essentially supporting the predictions based on tests and modeling.

  12. Non-collinear generation of angularly isolated circularly polarized high harmonics

    NASA Astrophysics Data System (ADS)

    Hickstein, Daniel D.; Dollar, Franklin J.; Grychtol, Patrik; Ellis, Jennifer L.; Knut, Ronny; Hernández-García, Carlos; Zusin, Dmitriy; Gentry, Christian; Shaw, Justin M.; Fan, Tingting; Dorney, Kevin M.; Becker, Andreas; Jaroń-Becker, Agnieszka; Kapteyn, Henry C.; Murnane, Margaret M.; Durfee, Charles G.

    2015-11-01

    We generate angularly isolated beams of circularly polarized extreme ultraviolet light through the first implementation of non-collinear high harmonic generation with circularly polarized driving lasers. This non-collinear technique offers numerous advantages over previous methods, including the generation of higher photon energies, the separation of the harmonics from the pump beam, the production of both left and right circularly polarized harmonics at the same wavelength and the capability of separating the harmonics without using a spectrometer. To confirm the circular polarization of the beams and to demonstrate the practicality of this new light source, we measure the magnetic circular dichroism of a 20 nm iron film. Furthermore, we explain the mechanisms of non-collinear high harmonic generation using analytical descriptions in both the photon and wave models. Advanced numerical simulations indicate that this non-collinear mixing enables the generation of isolated attosecond pulses with circular polarization.

  13. Extraordinary Second Harmonic Generation in Tungsten Disulfide Monolayers

    PubMed Central

    Janisch, Corey; Wang, Yuanxi; Ma, Ding; Mehta, Nikhil; Elías, Ana Laura; Perea-López, Néstor; Terrones, Mauricio; Crespi, Vincent; Liu, Zhiwen

    2014-01-01

    We investigate Second Harmonic Generation (SHG) in monolayer WS2 both deposited on a SiO2/Si substrate or suspended using transmission electron microscopy grids. We find unusually large second order nonlinear susceptibility, with an estimated value of deff ~ 4.5 nm/V nearly three orders of magnitude larger than other common nonlinear crystals. In order to quantitatively characterize the nonlinear susceptibility of two-dimensional (2D) materials, we have developed a formalism to model SHG based on the Green's function with a 2D nonlinear sheet source. In addition, polarized SHG is demonstrated as a useful method to probe the structural symmetry and crystal orientation of 2D materials. To understand the large second order nonlinear susceptibility of monolayer WS2, density functional theory based calculation is performed. Our analysis suggests the origin of the large nonlinear susceptibility in resonance enhancement and a large joint density of states, and yields an estimate of the nonlinear susceptibility value deff = 0.77 nm/V for monolayer WS2, which shows good order-of-magnitude agreement with the experimental result. PMID:24984953

  14. Third-harmonic generation susceptibility spectroscopy in free fatty acids

    NASA Astrophysics Data System (ADS)

    Chen, Yu-Cheng; Hsu, Hsun-Chia; Lee, Chien-Ming; Sun, Chi-Kuang

    2015-09-01

    Lipid-correlated disease such as atherosclerosis has been an important medical research topic for decades. Many new microscopic imaging techniques such as coherent anti-Stokes Raman scattering and third-harmonic generation (THG) microscopy were verified to have the capability to target lipids in vivo. In the case of THG microscopy, biological cell membranes and lipid bodies in cells and tissues have been shown as good sources of contrast with a laser excitation wavelength around 1200 nm. We report the THG excitation spectroscopy study of two pure free fatty acids including oleic acid and linoleic acid from 1090 to 1330 nm. Different pure fatty acids presented slightly-different THG χ(3) spectra. The measured peak values of THG third-order susceptibility χ(3) in both fatty acids were surprisingly found not to match completely with the resonant absorption wavelengths around 1190 to 1210 nm, suggesting possible wavelengths selection for enhanced THG imaging of lipids while avoiding laser light absorption. Along with the recent advancement in THG imaging, this new window between 1240 to 1290 nm may offer tremendous new opportunities for sensitive label-free lipid imaging in biological tissues.

  15. Imaging articular cartilage using second harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Mansfield, Jessica C.; Winlove, C. Peter; Knapp, Karen; Matcher, Stephen J.

    2006-02-01

    Sub cellular resolution images of equine articular cartilage have been obtained using both second harmonic generation microscopy (SHGM) and two-photon fluorescence microscopy (TPFM). The SHGM images clearly map the distribution of the collagen II fibers within the extracellular matrix while the TPFM images show the distribution of endogenous two-photon fluorophores in both the cells and the extracellular matrix, highlighting especially the pericellular matrix and bright 2-3μm diameter features within the cells. To investigate the source of TPF in the extracellular matrix experiments have been carried out to see if it may originate from the proteoglycans. Pure solutions of the following proteoglycans hyaluronan, chondroitin sulfate and aggrecan have been imaged, only the aggrecan produced any TPF and here the intensity was not great enough to account for the TPF in the extracellular matrix. Also cartilage samples were subjected to a process to remove proteoglycans and cellular components. After this process the TPF from the samples had decreased by a factor of two, with respect to the SHG intensity.

  16. Second harmonic generation from the ‘centrosymmetric’ crystals

    PubMed Central

    Nalla, Venkatram; Medishetty, Raghavender; Wang, Yue; Bai, Zhaozhi; Sun, Handong; Wei, Ji.; Vittal, Jagadese J.

    2015-01-01

    Second harmonic generation (SHG) is a well known non-linear optical phenomena which can be observed only in non-centrosymmetric crystals due to non-zero hyperpolarizability. In the current work we observed SHG from a Zn(II) complex which was originally thought to have crystallized in the centrosymmetric space group C2/c. This has been attributed to the unequal antiparallel packing of the metal complexes in the non-symmetric space group Cc or residual non-centrosymmetry in C2/c giving rise to polarizability leading to strong SHG. The enhancement of SHG by UV light has been attributed to the increase in non-centrosymmetry and hence polarity of packing due to strain induced in the crystals. The SHG signals measured from these crystals were as large as potassium dihydrogen phosphate crystals, KH2PO4 (KDP), and showed temperature dependence. The highest SHG efficiency was observed at 50 K. The SHG phenomenon was observed at broad wavelengths ranging from visible to below-red in these crystals. PMID:25995840

  17. Research of second harmonic generation images based on texture analysis

    NASA Astrophysics Data System (ADS)

    Liu, Yao; Li, Yan; Gong, Haiming; Zhu, Xiaoqin; Huang, Zufang; Chen, Guannan

    2014-09-01

    Texture analysis plays a crucial role in identifying objects or regions of interest in an image. It has been applied to a variety of medical image processing, ranging from the detection of disease and the segmentation of specific anatomical structures, to differentiation between healthy and pathological tissues. Second harmonic generation (SHG) microscopy as a potential noninvasive tool for imaging biological tissues has been widely used in medicine, with reduced phototoxicity and photobleaching. In this paper, we clarified the principles of texture analysis including statistical, transform, structural and model-based methods and gave examples of its applications, reviewing studies of the technique. Moreover, we tried to apply texture analysis to the SHG images for the differentiation of human skin scar tissues. Texture analysis method based on local binary pattern (LBP) and wavelet transform was used to extract texture features of SHG images from collagen in normal and abnormal scars, and then the scar SHG images were classified into normal or abnormal ones. Compared with other texture analysis methods with respect to the receiver operating characteristic analysis, LBP combined with wavelet transform was demonstrated to achieve higher accuracy. It can provide a new way for clinical diagnosis of scar types. At last, future development of texture analysis in SHG images were discussed.

  18. Titanosilicates with Strong Phase-Matched Second Harmonic Generation Responses.

    PubMed

    Chao, Tzu-Ling; Chang, Wen-Jung; Wen, Shu-Han; Lin, Yu-Qing; Chang, Bor-Chen; Lii, Kwang-Hwa

    2016-07-27

    The search for new and efficient nonlinear optical (NLO) materials has been an active research because of their technological importance in laser applications. Although a large number of frequency-doubling oxides, phosphates, borates, and fluoride-containing borates were found, no transition-metal silicate with useful NLO properties has been reported. We have now synthesized and grown crystals of two new titanosilicates, Li2K4[(TiO)Si4O12] and Li2Rb4[(TiO)Si4O12], by using a flux and supercritical hydrothermal method. Their unique 3D framework structures contain highly compressed TiO5 square pyramids which are arranged one over the other to form infinite ···Ti-O···Ti-O straight chains with alternating short and long Ti-O distances. These two materials meet the requirements for efficient second harmonic generation including lack of center of inversion symmetry, large susceptibility, phase matching, transmitting at wavelengths of interest, resistant to laser damage, and thermally stable. These attributes make them very attractive for frequency-doubling materials. PMID:27416357

  19. Second harmonic generation of chiral-modified silver nanoparticles

    NASA Astrophysics Data System (ADS)

    Tao, Yue; Aldea-Nunzi, Gabriela; Rao Bobbara, Sanyasi; Nunzi, Jean-Michel

    2013-10-01

    Various approaches for the optical detection of chiral compounds have been developed due to their natural optical activity. Since the advantages of second harmonic generation (SHG) on noble-metal nanoparticles (NPs) have been observed, it would be interesting to study the nonlinear phenomena from chiral compounds attached Ag NPs. In the present work, we fabricated chiral-modified Ag NPs based on the self-assembly process of cysteine and Ag, and carried out the investigation on SHG on modified and unmodified Ag NPs. For modified Ag NPs, either L-Cysteine (L-C) or D-Cysteine (D-C), as a pair of enantiomers, was applied on top of the Ag NPs. The resulting chiral-modified monolayers of L-C/Ag NPs and D-C/Ag NPs exhibit a reversed optical rotation difference (ORD) at linearly +/-45° polarization of SH, where no such difference exists for Ag NPs alone. SHG efficiently probes and discriminates L-C from D-C monolayers on the modified Ag NPs, which constitutes a simple and sensitive optical diagnostic of chiral molecules.

  20. Studies of surfaces using optical second-harmonic generation

    SciTech Connect

    Tom, H.W.K.

    1984-04-01

    The experiments reported in this thesis demonstrate the use of second-harmonic generation (SHG) and sum-frequency generation (SFG) in reflection from surfaces to study various surface properties. The experiments firmly establish SHG as a viable new surface probe that complements existing surface probes in ultrahigh vacuum environments and is in many ways unique for studying interfaces between dense media. Surface structural symmetry can be revealed through the anisotropy in the SH signal from the surface as the sample is rotated about its normal. The form of this anisotropy is derived in theory and verified with an experiment on the Si(100) and (111) surfaces. The SHG and SFG signals from molecules adsorbed on noninteracting substrates have a direct relationship to the number, average orientation, and spectroscopic properties of the molecules. The SH intensity was used to measure the isotherm for adsorption of p-nitrobenzoic acid from ethanolic solution to fused silica. Experiments performed on a strongly-interacting well-characterized Rh(111) surface in ultrahigh vacuum establish the sensitivity of the SH probe in corroboration with other surface probes. For the first time, the SH coverage-dependence was fit by theory in a quantitative way for the case of O-atom adsorption. The sensitivity of SH to adsorption at different sites was established for CO on top- and bridge-sites. SHG was shown to be surface specific in that the SHG from alkali metal surfaces originates from the first two monolayers. SH sensitivity to the adsorption of catalytically-important hydrocarbons and to chemical processes such as benzene dehydrogenation was also demonstrated. 122 references, 27 figures, 2 tables.

  1. Nonlinearly coupled localized plasmon resonances: Resonant second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Ginzburg, Pavel; Krasavin, Alexey; Sonnefraud, Yannick; Murphy, Antony; Pollard, Robert J.; Maier, Stefan A.; Zayats, Anatoly V.

    2012-08-01

    The efficient resonant nonlinear coupling between localized surface plasmon modes is demonstrated in a simple and intuitive way using boundary integral formulation and utilizing second-order optical nonlinearity. The nonlinearity is derived from the hydrodynamic description of electron plasma and originates from the presence of material interfaces in the case of small metal particles. The coupling between fundamental and second-harmonic modes is shown to be symmetry selective and proportional to the spatial overlap between polarization dipole density of the second-harmonic mode and the square of the polarization charge density of the fundamental mode. Particles with high geometrical symmetry will convert a far-field illumination into dark nonradiating second-harmonic modes, such as quadrupoles. Effective second-harmonic susceptibilities are proportional to the surface-to-volume ratio of a particle, emphasizing the nanoscale enhancement of the effect.

  2. Efficient second- and third-harmonic radiation generation from relativistic laser-plasma interactions

    SciTech Connect

    Singh, Mamta; Gupta, D. N.; Suk, H.

    2015-06-15

    We propose an idea to enhance the efficiency of second- and third-harmonic generation by considering the amplitude-modulation of the fundamental laser pulse. A short-pulse laser of finite spot size is modeled as amplitude modulated in time. Amplitude-modulation of fundamental laser contributes in quiver velocity of the plasma electrons and produces the strong plasma-density perturbations, thereby increase in current density at second- and third-harmonic frequency. In a result, the conversion efficiency of harmonic generation increases significantly. Power conversion efficiency of harmonic generation process is the increasing function of the amplitude-modulation parameter of the fundamental laser beam. Harmonic power generated by an amplitude modulated laser is many folds higher than the power obtained in an ordinary case.

  3. All-fiber fourth and fifth harmonic generation from a single source.

    PubMed

    Khudus, Muhammad I M Abdul; Lee, Timothy; De Lucia, Francesco; Corbari, Costantino; Sazio, Pier; Horak, Peter; Brambilla, Gilberto

    2016-09-19

    All-fiber fourth and fifth harmonic generation from a single source is demonstrated experimentally and analyzed theoretically. Light from a fully fiberized high power master oscillator power amplifier is launched into a periodically poled silica fiber generating the second harmonic. The output is then sent through two optical microfibers that generate the third and fourth harmonic, respectively, via four wave mixing (FWM). For a large range of pump wavelengths in the silica optical transmission window, phase matched FWM can be achieved in the microfibers at two different diameters with relatively wide fabrication tolerances of up to +/-5 nm. Our simulations indicate that by optimizing the second harmonic generation efficiency and the diameters and lengths of the two microfibers, conversion efficiencies to the fourth harmonic in excess of 25% are theoretically achievable. PMID:27661915

  4. Tracing the structure of asymmetric molecules from high-order harmonic generation

    SciTech Connect

    Chen Yanjun; Zhang, Bing

    2011-11-15

    We investigate high-order harmonic generation (HHG) from asymmetric molecules exposed to intense laser fields. We show that the emissions of odd and even harmonics depend differently on the orientation angle, the internuclear distance, as well as the effective charge. This difference mainly comes from different roles of intramolecular interference in the HHG of odd and even harmonics. These roles map the structure of the asymmetric molecule to the odd vs even HHG spectra.

  5. Characterization of muscle contraction with second harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Prent, Nicole

    Muscle cells have the ability to change length and generate force due to orchestrated action of myosin nanomotors that cause sliding of actin filaments along myosin filaments in the sarcomeres, the fundamental contractile units, of myocytes. The correlated action of hundreds of sarcomeres is needed to produce the myocyte contractions. This study probes the molecular structure of the myofilaments and investigates the movement correlations between sarcomeres during contraction. In this study, second harmonic generation (SHG) microscopy is employed for imaging striated myocytes. Myosin filaments in striated myocytes inherently have a nonzero second-order susceptibility, [special characters omitted] and therefore generate efficient SHG. Employing polarization-in polarization-out (PIPO) SHG microscopy allows for the accurate determination of the characteristic ratio, [special characters omitted] in birefringent myocytes, which describes the structure of the myosin filament. Analysis shows that the b value at the centre of the myosin filament, where the nonlinear dipoles are better aligned, is slightly lower than the value at the edges of the filament, where there is more disorder in orientation of the nonlinear dipoles from the myosin heads. Forced stretching of myocytes resulted in an SHG intensity increase with the elongation of the sarcomere. SHG microscopy captured individual sarcomeres during contraction, allowing for the measurement of sarcomere length (SL) and SHG intensity (SI) fluctuations. The fluctuations also revealed higher SHG intensity in elongated sarcomeres. The sarcomere synchronization model (SSM) for contracting and quiescent myocytes was developed, and experimentally verified for three cases (isolated cardiomyocyte, embryonic chicken cardiomyocyte, and larva myocyte). During contraction, the action of SLs and SIs between neighbouring sarcomeres partially correlated, whereas in quiescent myocytes the SLs show an anti-correlation and the SIs have no

  6. Studies of interfaces and vapors with Optical Second Harmonic Generation

    SciTech Connect

    Mullin, C. S.

    1993-12-01

    Optical Second Harmonic Generation (SHG) has been applied to the study of soap-like molecules adsorbed to the water-air interface. By calibrating the signal from a soluble monolayer with that of an insoluble homolog, absolute measurements of the surface density could be obtained and related to the bulk concentration and surface tension. We could then demonstrate that the soluble surfactant forms a single monolayer at the interface. Furthermore, it deviates significantly from the ideal case in that its activity coefficients are far from 1, yet those coefficients remain constant over a broad range of surface pressures. We present evidence of a first-order phase transition taking place during the adsorption of this soluble monolayer. We consider the effects of the non-ideal behavior and the phase transition on the microscopic model of adsorption, and formulate an alternative to the Langmuir picture of adsorption which is just as simple, yet it can more easily allow for non-ideal behavior. The second half of this thesis considers the problem of SHG in bulk metal vapors. The symmetry of the vapor forbids SHG, yet it has been observed. We consider several models whereby the symmetry of the vapor is broken by the presence of the laser and compare their predictions to new observations we have made using a few-picosecond laser pulse. The two-lobed output beam profile shows that it is the vapor-plus-beam combination whose symmetry is important. The dependence on vapor pressure demonstrates the coherent nature of the radiation, while the dependence on buffer gas pressure hints at a change of the symmetry in time. The time-dependence is measured directly with a preliminary pump-probe measurement. The magnitude and intensity dependence of the signal are also measured. All but one of the models are eliminated by this comparison.

  7. Second harmonic generation imaging microscopy of cellular structure and function

    NASA Astrophysics Data System (ADS)

    Millard, Andrew C.; Jin, Lei; Loew, Leslie M.

    2005-03-01

    Second harmonic generation (SHG) imaging microscopy is an important emerging technique for biological research, with many advantages over existing one- or two-photon fluorescence techniques. A non-linear phenomenon employing mode-locked Ti:sapphire or fiber-based lasers, SHG results in intrinsic optical sectioning without the need for a confocal aperture. Furthermore, as a second-order process SHG is confined to loci lacking a center of symmetry. Many important structural proteins such as collagen and cellulose show intrinsic SHG, thus providing access to sub-resolution information on symmetry. However, we are particularly interested here in "resonance-enhanced" SHG from styryl dyes. In general SHG is a combination of a true second-order process and a third-order process dependent on a static electric field, such that SHG from membrane-bound dyes depends on a cell's trans-membrane potential. With simultaneous patch-clamping and non-linear imaging of cells, we have found that SHG is a sensitive probe of trans-membrane potential with sensitivities that are up to four times better than those obtained under optimal conditions using one-photon fluorescence imaging. With the sensitivity of SHG to local electric fields from other sources such as the membrane dipole potential as well as the quadratic dependence of SHG on concentration, we have found that SHG imaging of styryl dyes is also a powerful technique for the investigation of lipid phases and rafts and for the visualization of the dynamics of membrane-vesicle fusion following fertilization of an ovum.

  8. Optical Second Harmonic Generation Studies of Electrochemical Interfaces

    NASA Astrophysics Data System (ADS)

    Nagy, Gabor

    Optical second harmonic generation (SHG) is an intrinsically surface sensitive tool that can be used to probe a wide variety of surface processes. In this work, SHG is employed to study the surface behavior of three polycrystalline electrodes, Cu, Ni, and brass, in an electrochemical environment. For the Cu electrode, SHG is used to examine the surface during oxidation and reduction in halide and non -halide electrolytes. The optical data indicate the probable formation of previously undetected small, resonant Cu clusters which are stabilized by Cu-halide crystallites on the electrode surface. The surface charge dependence of SHG is explored at a polycrystalline Ni electrode in the absence of faradaic reactions. The resulting correlation between surface charge and SHG indicates that in an electrochemical environment, the DC field activated contribution to the second order susceptibility plays the dominant role in SHG from Ni. Also with the polycrystalline Ni electrode, the behavior of the SH signal during the electrodeposition of Ag on the Ni surface is examined. The analysis of the optical data in conjunction with a diffusion limited Ag island growth model indicates that the SH signal experiences an electromagnetic enhancement on the Ni surface as a result of the Ag islands. The charge dependence of the SH signal is examined on a polycrystalline alpha-brass electrode in the absence of faradaic reactions, with two incident wavelengths. The experiments show that, as is the case with Cu, SHG from brass may (depending on the incident wavelength) also involve an interband transition and can be affected by a charge dependent Stark shift of the interband transition threshold. The brass electrode is also examined with SHG in a potential region where the selective dissolution of the surface Zn sites is known to occur. By using a layer-by-layer reordering model of the dissolving surface, the electrochemical data is correlated with simultaneously obtained optical SHG data to

  9. The Galileo high gain antenna deployment anomaly

    NASA Technical Reports Server (NTRS)

    Johnson, Michael R.

    1994-01-01

    On April 11, 1991, the Galileo spacecraft executed a sequence that would open the spacecraft's High Gain Antenna. The Antenna's launch restraint had been released just after deployment sequence, the antenna, which opens like an umbrella, never reached the fully deployed position. The analyses and tests that followed allowed a conclusive determination of the likely failure mechanisms and pointed to some strategies to use for recovery of the high gain antenna.

  10. Oriented rotational wave-packet dynamics studies via high harmonic generation.

    PubMed

    Frumker, E; Hebeisen, C T; Kajumba, N; Bertrand, J B; Wörner, H J; Spanner, M; Villeneuve, D M; Naumov, A; Corkum, P B

    2012-09-14

    We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wave packet is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the wave packet, generating even-order high harmonics that arise from the broken symmetry induced by the orientation dynamics. The even-order harmonic radiation that we measure appears on a zero background, enabling us to accurately follow the temporal evolution of the wave packet. Our measurements reveal that, for the conditions optimum for harmonic generation, the orientation is produced by preferential ionization which depletes the sample of molecules of one orientation. PMID:23005628

  11. Second harmonic generation in nanoscale films of transition metal chalcogenides: Taking into account multibeam interference

    NASA Astrophysics Data System (ADS)

    Lavrov, S. D.; Kudryavtsev, A. V.; Shestakova, A. P.; Kulyuk, L.; Mishina, E. D.

    2016-05-01

    Second harmonic generation is studied in structures containing nanoscale layers of transition metal chalcogenides that are two-dimensional semiconductors and deposited on a SiO2/Si substrate. The second harmonic generation intensity is calculated with allowance for multibeam interference in layers of dichalcogenide and silicon oxide. The coefficient of reflection from the SiO2-layer-based Fabry-Perot cavity is subsequently calculated for pump wave fields initiating nonlinear polarization at every point of dichalcogenide, which is followed by integration of all second harmonic waves generated by this polarization. Calculated second harmonic intensities are presented as functions of dichalcogenide and silicon oxide layer thicknesses. The dependence of the second harmonic intensity on the MoS2 layer thickness is studied experimentally in the layer of 2-140 nm. A good coincidence of the experimental data and numerical simulation results has been obtained.

  12. Effect of nuclear motion on spectral broadening of high-order harmonic generation.

    PubMed

    Yuan, Xiaolong; Wei, Pengfei; Liu, Candong; Ge, Xiaochun; Zheng, Yinghui; Zeng, Zhinan; Li, Ruxin

    2016-04-18

    High-order harmonic generation (HHG) in molecular targets is experimentally investigated in order to reveal the role of the nuclear motion played in the harmonic generation process. An obvious broadening in the harmonic spectrum from the H2 molecule is observed in comparison with the harmonic spectrum generated from other molecules with relatively heavy nuclei. We also find that the harmonic yield from the H2 molecule is much weaker than the yield from those gas targets with the similar ionization potentials, such as Ar atom and N2 molecule. The yield suppression and the spectrum broadening of HHG can be attributed to the vibrational motion of nuclear induced by the driving laser pulse. Moreover, the one-dimensional (1D) time-dependent Schrödinger equation (TDSE) with the non-Born-Oppenheimer (NBO) treatment is numerically solved to provide a theoretical support to our explanation.

  13. Enhanced third harmonic generation in air by two-colour ultrashort laser pulses

    NASA Astrophysics Data System (ADS)

    Nath, Arpita; Dharmadhikari, J. A.; Mathur, D.; Dharmadhikari, A. K.

    2016-09-01

    We report on third harmonic generation in air in a non-filamentation regime using tightly focused, ultrashort laser pulses (1-2 µm wavelength). Enhancement in the third harmonic efficiency is observed from co-propagating laser pulses of two different wavelengths which emanate from the same source—an optical parametric amplifier—and are spatially and temporally overlapped. The third harmonic efficiency for signal wavelength (1.35 µm) is measured to be 4 × 10-3 %; in the presence of idler wavelength (2.09 µm), the corresponding value becomes 1.6 × 10-2 %—a fourfold enhancement in efficiency. The pulse duration of the generated third harmonic is measured to be 37 fs. We examine the possible role of plasma to account for the observed enhancement in third harmonic generation.

  14. Effect of nuclear motion on spectral broadening of high-order harmonic generation.

    PubMed

    Yuan, Xiaolong; Wei, Pengfei; Liu, Candong; Ge, Xiaochun; Zheng, Yinghui; Zeng, Zhinan; Li, Ruxin

    2016-04-18

    High-order harmonic generation (HHG) in molecular targets is experimentally investigated in order to reveal the role of the nuclear motion played in the harmonic generation process. An obvious broadening in the harmonic spectrum from the H2 molecule is observed in comparison with the harmonic spectrum generated from other molecules with relatively heavy nuclei. We also find that the harmonic yield from the H2 molecule is much weaker than the yield from those gas targets with the similar ionization potentials, such as Ar atom and N2 molecule. The yield suppression and the spectrum broadening of HHG can be attributed to the vibrational motion of nuclear induced by the driving laser pulse. Moreover, the one-dimensional (1D) time-dependent Schrödinger equation (TDSE) with the non-Born-Oppenheimer (NBO) treatment is numerically solved to provide a theoretical support to our explanation. PMID:27137258

  15. Third harmonic generation in air ambient and laser ablated carbon plasma

    SciTech Connect

    Singh, Ravi Pratap Gupta, Shyam L.; Thareja, Raj K.

    2015-12-15

    We report the third harmonic generation of a nanosecond laser pulse (1.06 μm) in air ambient and in the presence of nanoparticles from laser ablated carbon plasma. Significant decrease in the threshold of third harmonic generation and multi-fold increment in the intensity of generated third harmonic is observed in presence of carbon plasma. The third harmonic in air is due to the quasi-resonant four photon process involving vibrationally excited states of molecular ion of nitrogen due to electron impact ionization and laser pulse. Following optical emission spectroscopic observations we conclude that the presence of C{sub 2} and CN in the ablated plume play a vital role in the observed third harmonic signals.

  16. Resonant second harmonic generation in a gallium nitride two-dimensional photonic crystal on silicon

    SciTech Connect

    Zeng, Y.; Roland, I.; Checoury, X.; Han, Z.; El Kurdi, M.; Sauvage, S.; Boucaud, P.; Gayral, B.; Brimont, C.; Guillet, T.; Mexis, M.; Semond, F.

    2015-02-23

    We demonstrate second harmonic generation in a gallium nitride photonic crystal cavity embedded in a two-dimensional free-standing photonic crystal platform on silicon. The photonic crystal nanocavity is optically pumped with a continuous-wave laser at telecom wavelengths in the transparency window of the nitride material. The harmonic generation is evidenced by the spectral range of the emitted signal, the quadratic power dependence vs. input power, and the spectral dependence of second harmonic signal. The harmonic emission pattern is correlated to the harmonic polarization generated by the second-order nonlinear susceptibilities χ{sub zxx}{sup (2)}, χ{sub zyy}{sup (2)} and the electric fields of the fundamental cavity mode.

  17. Enhancing High-Order Harmonic Generation in Light Molecules by Using Chirped Pulses.

    PubMed

    Lara-Astiaso, M; Silva, R E F; Gubaydullin, A; Rivière, P; Meier, C; Martín, F

    2016-08-26

    One of the current challenges in high-harmonic generation is to extend the harmonic cutoff to increasingly high energies while maintaining or even increasing the efficiency of the high-harmonic emission. Here we show that the combined effect of down-chirped pulses and nuclear dynamics in light molecules allows one to achieve this goal, provided that long enough IR pulses are used to allow the nuclei to move well outside the Franck-Condon region. We also show that, by varying the duration of the chirped pulse or by performing isotopic substitution while keeping the pulse duration constant, one can control the extension of the harmonic plateau. PMID:27610851

  18. Enhancing High-Order Harmonic Generation in Light Molecules by Using Chirped Pulses

    NASA Astrophysics Data System (ADS)

    Lara-Astiaso, M.; Silva, R. E. F.; Gubaydullin, A.; Rivière, P.; Meier, C.; Martín, F.

    2016-08-01

    One of the current challenges in high-harmonic generation is to extend the harmonic cutoff to increasingly high energies while maintaining or even increasing the efficiency of the high-harmonic emission. Here we show that the combined effect of down-chirped pulses and nuclear dynamics in light molecules allows one to achieve this goal, provided that long enough IR pulses are used to allow the nuclei to move well outside the Franck-Condon region. We also show that, by varying the duration of the chirped pulse or by performing isotopic substitution while keeping the pulse duration constant, one can control the extension of the harmonic plateau.

  19. Experimental observation of cumulative second-harmonic generation of lamb waves propagating in long bones.

    PubMed

    Zhang, Zhenggang; Liu, Dan; Deng, Mingxi; Ta, Dean; Wang, Weiqi

    2014-07-01

    The experimental observation of cumulative second-harmonic generation of fundamental Lamb waves in long bones is reported. Based on the modal expansion approach to waveguide excitation and the dispersion characteristics of Lamb waves in long bones, the mechanism underlying the generation and accumulation of second harmonics by propagation of the fundamental Lamb waves was investigated. An experimental setup was established to detect the second-harmonic signals of Lamb wave propagation in long bones in vitro. Through analysis of the group velocities of the received signals, the appropriate fundamental Lamb wave modes and the duration of the second-harmonic signals could be identified. The integrated amplitude of the time-domain second-harmonic signal was introduced and used to characterize the efficiency of second-harmonic generation by fundamental Lamb wave propagation. The results indicate that the second-harmonic signal generated by fundamental Lamb waves propagating in long bones can be observed clearly, and the effect was cumulative with propagation distance when the fundamental Lamb wave mode and the double-frequency Lamb wave mode had the same phase velocities. The present results may be important in the development of a new method to evaluate the status of long bones using the cumulative second harmonic of ultrasonic Lamb waves.

  20. Second-harmonic generation with pulses in a coupled-resonator optical waveguide.

    PubMed

    Mookherjea, Shayan; Yariv, Amnon

    2002-02-01

    We describe the generation and propagation of pulses in a coupled-resonator optical waveguide driven by a nonlinear polarization using a method closely related to the coupled-mode theory. The specific example we consider is that of second-harmonic generation. This formalism explicitly accounts for temporal dependencies in the waveguide field distributions and in their representations in terms of slowly modulated Bloch wave functions, in contrast with the equations obtained previously for cw second-harmonic generation.

  1. Spatial properties of odd and even low order harmonics generated in gas

    PubMed Central

    Lambert, G.; Andreev, A.; Gautier, J.; Giannessi, L.; Malka, V.; Petralia, A.; Sebban, S.; Stremoukhov, S.; Tissandier, F.; Vodungbo, B.; Zeitoun, Ph.

    2015-01-01

    High harmonic generation in gases is developing rapidly as a soft X-ray femtosecond light-source for applications. This requires control over all the harmonics characteristics and in particular, spatial properties have to be kept very good. In previous literature, measurements have always included several harmonics contrary to applications, especially spectroscopic applications, which usually require a single harmonic. To fill this gap, we present here for the first time a detailed study of completely isolated harmonics. The contribution of the surrounding harmonics has been totally suppressed using interferential filtering which is available for low harmonic orders. In addition, this allows to clearly identify behaviors of standard odd orders from even orders obtained by frequency-mixing of a fundamental laser and of its second harmonic. Comparisons of the spatial intensity profiles, of the spatial coherence and of the wavefront aberration level of 5ω at 160 nm and 6ω at 135 nm have then been performed. We have established that the fundamental laser beam aberrations can cause the appearance of a non-homogenous donut-shape in the 6ω spatial intensity distribution. This undesirable effect can be easily controlled. We finally conclude that the spatial quality of an even harmonic can be as excellent as in standard generation. PMID:25585715

  2. Preparation and second-harmonic generation in Pb-doped oxide glasses

    NASA Astrophysics Data System (ADS)

    Liu, Qiming; Wang, Mingliang; Zhao, Xiujian

    2008-12-01

    PbO-B2O3 glasses were prepared by traditional melting method. XRD and optical spectra measurements were done to check properties. Second-harmonic generation was observed in the glasses induced by thermal treatment and thermally poling process, respectively. But second-harmonic generation intensity was normally larger for the later, and it increased with increasing PbO content, poling voltage, temperature and time. The mechanism of second-harmonic generation in the PbO-B2O3 glasses was also discussed. A promising material for all-optical switching devices is expected.

  3. Second harmonic generation in ZnO thin films fabricated by metalorganic chemical vapor deposition

    NASA Astrophysics Data System (ADS)

    Liu, C. Y.; Zhang, B. P.; Binh, N. T.; Segawa, Y.

    2004-07-01

    Second harmonic generation (SHG) from ZnO thin films fabricated by metalorganic chemical vapor deposition (MOCVD) technique was carried out. By comparing the second harmonic signal generated in a series of ZnO films with different deposition temperatures, we conclude that a significant part of second harmonic signal is generated at the film deposited with appropriate temperature. The second-order susceptibility tensor χ(2)zzz=9.2 pm/V was deduced for a film deposited at 250 °C.

  4. Nonlinearly generated harmonic signals in ultra-small waveguides with magnetic films: Tunable enhancements of 2nd and 4th harmonics

    NASA Astrophysics Data System (ADS)

    Marsh, J.; Zagorodnii, V.; Celinski, Z.; Camley, R. E.

    2012-03-01

    The nonlinear generation of high harmonic signals (up to 5th harmonic) is explored in an ultra-small waveguide which contains a thin ferromagnetic film. The strength of the different harmonics is highly tunable. In particular, the power in the 2nd and 4th harmonic signals may be enhanced by over two orders of magnitude by varying the direction of a static magnetic field with respect to the long axis of the waveguide. In contrast, the 3rd and 5th harmonics are relatively insensitive to the direction of the magnetic field. The experimental results are explained by analytical and numerical calculations.

  5. Signatures of symmetry and electronic structure in high-order harmonic generation in polyatomic molecules

    SciTech Connect

    Wong, M. C. H.; Brichta, J.-P.; Bhardwaj, V. R.

    2010-06-15

    We report detailed measurements of high-order harmonic generation in chloromethane molecules (CCl{sub 4}, CHCl{sub 3}, and CH{sub 2}Cl{sub 2}) to show that fingerprints of symmetry and electronic structure can be decoded from high-order harmonic generation even in complex randomly oriented molecules. In our measurements, orbital symmetries of these molecules are manifested as both extended harmonic cutoffs and a local minimum in the ellipticity dependence of the cut-off harmonics, suggesting the occurrence of quantum interferences during ionization. The harmonic spectra exhibit distinct interference minima at {approx}42 and {approx}60 eV. We attribute the former to the Cooper minimum in the photoionization cross section and the latter to intramolecular interference during the recombination process.

  6. Two-color high-harmonic generation in plasmas: efficiency dependence on the generating particle properties.

    PubMed

    Emelina, Anna S; Emelin, Mikhail Yu; Ganeev, Rashid A; Suzuki, Masayuki; Kuroda, Hiroto; Strelkov, Vasily V

    2016-06-27

    The high-order harmonic generation (HHG) in silver, gold, and zinc plasma plumes irradiated by orthogonally polarized two-color field is studied theoretically and experimentally. We find an increase of the HHG efficiency in comparison with the single-color case, which essentially depends on the plasma species and harmonic order. An increase of more than an order of magnitude is observed for silver plasma, whereas for gold and zinc it is lower; these results are reproduced in our calculations that include both propagation and microscopic response studies. We show that the widely used theoretical approach assuming the 1s ground state of the generating particle fails to reproduce the experimental results; the agreement is achieved in our theory using the actual quantum numbers of the outer electron of the generating particles. Moreover, our theoretical studies highlight the redistribution of the electronic density in the continuum wave packet as an important aspect of the HHG enhancement in the two-color orthogonally polarized fields with comparable intensities: in the single-color field the electronic trajectories with almost zero return energy are the most populated ones; in the two-color case the total field maximum can be shifted in time so that the trajectories with high return energies (in particular, the cut-off trajectory) become the most populated ones. PMID:27410560

  7. Systematic Review and Harmonization of Life Cycle GHG Emission Estimates for Electricity Generation Technologies (Presentation)

    SciTech Connect

    Heath, G.

    2012-06-01

    This powerpoint presentation to be presented at the World Renewable Energy Forum on May 14, 2012, in Denver, CO, discusses systematic review and harmonization of life cycle GHG emission estimates for electricity generation technologies.

  8. Frequency-resolved optical grating using surface third-harmonic generation

    SciTech Connect

    Tsang, T.; Krumbuegel, M.A.; Delong, K.W.; Fittinghoff, D.N.; Trebino, R.

    1995-11-01

    We demonstrate the frequency-resolved optical grating technique using third-harmonic generation on the surface of a cover glass with ultra-short optical pulses and compare that with the phase-retrieved spectrogram.

  9. Low-order harmonic generation in metal ablation plasmas in nanosecond and picosecond laser regimes

    SciTech Connect

    Lopez-Arias, M.; Oujja, M.; Sanz, M.; Castillejo, M.; Ganeev, R. A.; Boltaev, G. S.; Satlikov, N. Kh.; Tugushev, R. I.; Usmanov, T.

    2012-02-15

    Low-order harmonics, third and fifth, of IR (1064 nm) laser emission have been produced in laser ablation plasmas of the metals manganese, copper and silver. The harmonics were generated in a process triggered by laser ablation followed by frequency up-conversion of a fundamental laser beam that propagates parallel to the target surface. These studies were carried out in two temporal regimes by creating the ablation plasma using either nanosecond or picosecond pulses and then probing the plasma plume with pulses of the same duration. The spatiotemporal behavior of the generated harmonics was characterized and reveals the distinct composition and dynamics of the plasma species that act as nonlinear media, allowing the comparison of different processes that control the generation efficiency. These results serve to guide the choice of laser ablation plasmas to be used for efficient high harmonic generation of laser radiation.

  10. Generation of ultra-intense gamma-ray train by QED harmonics

    NASA Astrophysics Data System (ADS)

    Liu, Chen; Shen, Baifei; Zhang, Xiaomei; Ji, Liangliang; Wang, Wenpeng; Xu, Jiancai; Zhao, Xueyan; Yi, Longqing; Shi, Yin; Zhang, Lingang; Xu, Tongjun; Pei, Zhikun; Xu, Zhizhan

    2016-08-01

    In nonlinear media, photons may combine into a photon of energy and momentum of all those photons. This process, called harmonic generation, happens in nonlinear crystal, gas, and relativistic plasma. When the laser intensity reaches 1022 W/cm2, QED effects appear and play a significant role in the harmonic generation. In contrast to the gas and relativistic high-order harmonic generation processes, harmonics influenced by QED effects are usually not coherent because of the characteristic of random radiation, while the property of high intensity and ultra-short duration is conserved. In this work, the generation of high-order harmonics with QED effects is investigated by one- and two-dimensional particle-in-cell simulations. Studies have shown that interacting with a laser pulse with the intensity of I =5.35 ×1023W /cm 2 , such harmonics can produce ultra-short gamma-ray train with periodic structures. The period of gamma-ray train is half of the laser period, and the peak intensity is 1.4 ×1022W /cm 2 from one-dimensional simulation when ions are considered immobile. This new harmonic production with QED effects are crucial to light-matter interaction in strong field and can be verified in experiments by 10 PW laser facilities in the near future.

  11. Phase-matched second harmonic generation with on-chip GaN-on-Si microdisks

    PubMed Central

    Roland, I.; Gromovyi, M.; Zeng, Y.; El Kurdi, M.; Sauvage, S.; Brimont, C.; Guillet, T.; Gayral, B.; Semond, F.; Duboz, J. Y.; de Micheli, M.; Checoury, X.; Boucaud, P.

    2016-01-01

    We demonstrate phase-matched second harmonic generation in gallium nitride on silicon microdisks. The microdisks are integrated with side-coupling bus waveguides in a two-dimensional photonic circuit. The second harmonic generation is excited with a continuous wave laser in the telecom band. By fabricating a series of microdisks with diameters varying by steps of 8 nm, we obtain a tuning of the whispering gallery mode resonances for the fundamental and harmonic waves. Phase matching is obtained when both resonances are matched with modes satisfying the conservation of orbital momentum, which leads to a pronounced enhancement of frequency conversion. PMID:27687007

  12. High-order harmonic generation of picosecond radiation of moderate intensity in laser plasma

    SciTech Connect

    Boltaev, G S; Ganeev, Rashid A; Kulagin, I A; Satlikov, N Kh; Usmanov, T

    2012-10-31

    The results of investigations into the generation of highorder harmonics (up to the 21st order) of picosecond ({tau} = 38 ps) Nd : YAG laser radiation in the plasma produced by laser ablation of metal and carbon-containing material surfaces are presented. We demonstrate the feasibility of generating high-order harmonics in the vacuum ultraviolet spectral range (with radiation wavelengths shorter than 120 nm) in plasmas with an efficiency of {approx}0.7 Multiplication-Sign 10{sup -4}. In carbon-containing plasma, the 7th harmonic intensity exceeded that of the 5th one by a factor of seven. (nonlinear optical phenomena)

  13. High-order harmonic generation of picosecond radiation of moderate intensity in laser plasma

    NASA Astrophysics Data System (ADS)

    Boltaev, G. S.; Ganeev, Rashid A.; Kulagin, I. A.; Satlikov, N. Kh; Usmanov, T.

    2012-10-01

    The results of investigations into the generation of highorder harmonics (up to the 21st order) of picosecond (τ = 38 ps) Nd : YAG laser radiation in the plasma produced by laser ablation of metal and carbon-containing material surfaces are presented. We demonstrate the feasibility of generating high-order harmonics in the vacuum ultraviolet spectral range (with radiation wavelengths shorter than 120 nm) in plasmas with an efficiency of ~0.7 × 10-4. In carbon-containing plasma, the 7th harmonic intensity exceeded that of the 5th one by a factor of seven.

  14. Harmonic generation during ultrashort-pulse ultraintense /p-polarized laser interaction with solid target

    NASA Astrophysics Data System (ADS)

    Wu, Shuai; Zhan, Ru-Juan; Chen, Ji

    2001-07-01

    In this Letter, we developed the “relativistic surface currents” model to investigate the harmonic generation under the conditions of p-polarized obliquely incident ultrashort-pulse ultraintense laser. As a result of this Letter, up to 70 harmonics are generated with conversion efficiencies exceeding 10 -6, which is very close to the result from Norreys' experiment and Gibbon's PIC simulations. For highly relativistic regime and nonrelativistic regime of laser power, the harmonic conversion efficiencies as a function of laser strength parameter q are discussed.

  15. Very high gain Nd:YLF amplifiers

    SciTech Connect

    Knights, M.G.; Thomas, M.D.; Chicklis, E.P.; Rines, G.A.; Seka, W.

    1988-05-01

    The authors report on high gain Nd:YLF rod amplifiers in which single-pass, small signal gains of over 1700 have been obtained along with stored energy densitiesgreater than or equal to0.4J/cm/sup 3/. The ability of Nd:YLF amplifiers to support such gains is a result of high parasitic oscillation thresholds, due primarily to the low refractive index of the material. These results suggest that Nd:YLF is an excellent candidate for amplifiers where high specific stored energies and/or very high gains are required.

  16. Second harmonic generation from direct band gap quantum dots pumped by femtosecond laser pulses

    SciTech Connect

    Liu, Liwei Wang, Yue; Hu, Siyi; Ren, Yu; Huang, Chen

    2014-02-21

    We report on nonlinear optical experiments performed on Cu{sub 2}S quantum dots (QDs) pumped by femtosecond laser pulses. We conduct a theoretical simulation and experiments to determine their second harmonic generation characteristics. Furthermore, we demonstrate that the QDs have a second harmonic generation conversion efficiency of up to 76%. Our studies suggest that these Cu{sub 2}S QDs can be used for solar cells, bioimaging, biosensing, and electric detection.

  17. Raman parametric excitation effect upon the third harmonic generation by a metallic nanoparticle lattice

    SciTech Connect

    Sepehri Javan, N.

    2015-08-21

    This work is a theoretical study on third harmonic generation in the nonlinear propagation of an intense laser pulse through a periodic three-dimensional lattice of nanoparticles. Using a perturbative method, the nonlinear equations that describe the laser–nanoparticle interaction in the weakly relativistic regime are derived. Additionally, the nonlinear dispersion relation and the amplitude of the third harmonic are obtained. Finally, the effects of the nanoparticle radius and separation length, the distribution of the nanoparticle electron density, and the laser frequency upon the third harmonic efficiency are investigated. In addition to the expected resonance that occurs when the third harmonic resonates with the plasmon wave, another resonance appears when the nonlinear interaction of the fundamental mode with the third harmonic excites a longitudinal collective plasmon wave via the parametric Raman mechanism.

  18. Higher and sub-harmonic Lamb wave mode generation due to debond-induced contact nonlinearity

    NASA Astrophysics Data System (ADS)

    Guha, Anurup; Bijudas, C. R.

    2016-04-01

    Non-cumulative higher and sub-harmonic Lamb wave mode generation as a result of partial-debond of piezoelectric wafer transducers (PWT) bonded onto an Aluminium plate, is numerically investigated and experimentally validated. The influence of excitation frequency on the extent of nonlinearity due to clapping mechanism of the partially-debonded PWTs is discussed. A set of specific frequency range is arrived at based on the Eigen-value and Harmonic analyses of PWTs used in the model. It is found that, at these frequencies, which are integral multiple of the first width-direction mode of a PWT, significantly higher amplitudes of higher-harmonics are observed. It is also seen that at specific debond-positions and lengths, sharp sub-harmonics in addition to higher-harmonics are present. Signal processing is carried out using Fast Fourier transform, which is normalized for comparisons.

  19. High-order harmonic generation in the presence of a static electric field

    SciTech Connect

    Odzak, S.; Milosevic, D.B.

    2005-09-15

    We consider high-order harmonic generation by a linearly polarized laser field and a parallel static electric field. We first develop a modified saddle-point method which enables a quantitative analysis of the harmonic spectra even in the presence of Coulomb singularities. We introduce a classification of the saddle-point solutions and show that, in the presence of a static electric field which breaks the inversion symmetry, an additional classification number has to be introduced and that the usual saddle-point approximation and the uniform approximation in the case of the coalescing saddle points have to be modified. The theory developed offers a simple and accurate explanation of the static-field-induced multiplateau structure of the harmonic spectra. The longer quantum orbits are responsible for a long extension of the harmonic plateau, while the larger initial electron velocities are the reason of lower harmonic emission rates.

  20. Ultrahigh harmonics generation in a FEL with a seed laser

    SciTech Connect

    Goloviznin, V.V.; Amersfoort, P.W. van

    1995-12-31

    One of the most challenging problems in modern FEL technology is to operate in the X-ray region, especially in the {open_quotes}water window{close_quotes}. Because of the absence of optical resonators in this range of wavelengths, only a single-pass device may be suitable for this task. The Self-Amplified Spontaneous Emission (SASE) mechanism is now under active discussion as a realistic way to provide high-power coherent emission in the X-ray range. Both the undulator parameters and the electron beam parameters required for the lasing are achieveable at today`s technological level. On the other hand, the SASE approach implies a very long and expensive periodic magnetic structure, typically several tens of meters long. This is mainly because of the rather long build-up time necessary to establish a coherent mode from incoherent noise. A mechanism of shortening this time would be therefore highly desirable. In the present paper we consider a scheme using two undulators and a seed-laser to produce coherent X-ray emission. The first undulator and the seed-laser provide a pre-modulation of the beam while the second undulator serves as a source of coherent spontaneous radiation at a very high harmonic of the seed-laser frequency; the whole scheme may then be considered to be an FEL-based frequency upconvertor. The total length of the periodic magnetic structure is shown to be of the order of several meters, nearly an order of magnitude shorter than in the SASE case. For the same beam quality as in the SASE scheme and with realistic seed-laser parameters, the efficiency of the beam pre-modulation at the 50-th (!) harmonic is shown to be as high as 15%. The output radiation is tunable between discrete harmonics of the seed-frequency.

  1. Coherent and incoherent second harmonic generation in liquids

    NASA Astrophysics Data System (ADS)

    Maurice, A.; Benichou, E.; Brevet, P. F.

    2015-08-01

    In this paper, the Second Harmonic light intensity scattered off a liquid solution upon illumination by an incident fundamental frequency beam is written within a general framework in order to describe its coherent and incoherent contributions. It is shown that this formulation requires the introduction of a correlation function in time, position and orientation. We discuss this framework in light of recent experiments where the interface and the bulk of liquid solutions can be investigated simultaneously. We apply here this analysis to a neat water solution to compare the bulk volume and the interface correlation functions.

  2. Two-color probe of high harmonic generation from argon atoms

    NASA Astrophysics Data System (ADS)

    Zhao, Zengxiu; Yuan, Jianmin; Meng, Chao; Chen, Wenbo

    2014-05-01

    Two-color control of high harmonic generation has been proven a powerful in situ tool to characterize the intrinsic chirp of attosecond bursts. The weak second harmonic pulse introduces a phase modulation of the strong field quantum processes, leading to the generation of even-order harmonic. We measure the yields of even-order harmonics from argon gases as a function of the phase delay between the fundamental and its second harmonic pulse. We found that the modulation of even-order harmonics exhibits a phase jump around the 28th harmonic (48eV), closely resembling the result from. However, we show by varying laser intensity that the phase jump is unlikely to be attributed to the switching from short to long trajectories of HHG near the cut-off. In addition, we demonstrate that the phase of jump depends on the driving laser wavelength. Single-active-electron simulation fails to reproduce the experimental observation. We therefore suspect that multielectron response comes into play for the two-color control of HHG from Argon. Preliminary analysis suggests that there exists competing pathways of HHG from inner orbitals, even for argon atoms whose interaction with strong laser fields is usually assumed well described by SAE approximation.

  3. Theoretical analysis of high-order harmonic generation from a coherent superposition of states

    SciTech Connect

    Milosevic, Dejan B.

    2006-02-15

    A quantum theory of high-order harmonic generation by a strong laser field in the presence of more bound states is formulated. The obtained numerical and analytical results for a two-state hydrogenlike atom model show that the harmonic spectrum consists of two parts: a usual single-state harmonic spectrum of odd harmonics having the energies (2k+1){omega} and a resonant part with the peaks around the excitation energy {delta}{omega}. The energy of the harmonics in the resonant part of the spectrum is equal to {delta}{omega}{+-}{omega}, {delta}{omega}{+-}3{omega}, .... For energies higher than the excitation energy, the resonant part forms a plateau, followed by a cutoff. The emission rate of the harmonics in this resonant plateau is many orders of magnitude higher than that of the harmonics generated in the presence of the ground state alone. The influence of the depletion of the initial states, as well as of the pulse shape and intensity, is analyzed.

  4. Generation of higher-order harmonics from solid targets irradiated with fs-laser pulses

    NASA Astrophysics Data System (ADS)

    Tsakiris, G. D.

    1998-11-01

    The prospect of laser intensities exceeding the 10^19 W/cm^2 level becoming available from table-top, 10 Hz lasers, has given new impetus to the subject of solid harmonics [1]. After the initial experiments demonstrating the feasibility of harmonic generation with fs-laser pulses [2], the current effort is directed towards finding out the link between relevant plasma parameters and harmonic generation. The questions that arise are what are the limitations inherent to the generation mechanism and how one can optimize the harmonic yield. For example, in experiments using the Ti:sapphire laser ATLAS at Max-Planck Institut für Quantenoptik [3], it was found that the lower the contrast of the laser pulse the weaker the Iλ^2 scaling of the harmonic conversion efficiency. Some of these results are presented and their implications to solid harmonic generation at higher intensities will be discussed. [1] P. Gibbon, IEEE J. of Q. Elec. 33, 1915 (1997). [2] S. Kohlweyer, et al., Optics Comm. 177, 431 (1995). [3] M. Zepf, et al., submitted for publication in Phys. Rev. Lett.

  5. Surface plasma wave assisted second harmonic generation of laser over a metal film

    SciTech Connect

    Chauhan, Santosh; Parashar, J.

    2015-01-15

    Second harmonic generation of laser mode converted surface plasma wave (SPW) over a corrugated metal film is studied. The laser, impinged on the metal film, under attenuated total reflection configuration, excites SPW over the metal–vacuum interface. The excited SPW extends over a much wider surface area than the laser spot cross-section. It exerts a second harmonic ponderomotive force on metal electrons, imparting them velocity that beats with the surface ripple to produce a nonlinear current, driving resonant second harmonic surface plasma wave.

  6. Generation of high-power tunable terahertz-radiation by nonrelativistic beam-echo harmonic effect

    NASA Astrophysics Data System (ADS)

    Gong, Huarong; Travish, Gil; Xu, Jin; Wei, Yanyu; Feng, Jinjun; Gong, Yubin

    2013-01-01

    A new type of terahertz radiation source based on the nonrelativistic electron beam-wave interaction is proposed. Here, the beam echo harmonic effect is applied to a traveling wave tube like device. The scheme is configured as a combination of a frequency multiplier and amplifier with, for instance, W-band (millimeter wave) input signals and terahertz output power. A one-dimensional model of this device shows that a 10th order harmonic-wave can be generated while other harmonic waves are suppressed. The device only requires a readily available input source (W-band), and the output frequency can be tuned continuously over a wide band.

  7. Seventh-harmonic generation from tightly focused 2 μm ultrashort pulses in air.

    PubMed

    Nath, Arpita; Dharmadhikari, Jayashree A; Dharmadhikari, Aditya K; Mathur, Deepak

    2013-07-15

    We report generation of third, fifth and seventh harmonics from air by using tightly focused, ultrashort pulses of short-wave infrared (2 μm) radiation. We have measured the third- and fifth-harmonic efficiencies to be 5×10(-5) and ~1.4×10(-5), respectively, with the ratio of fifth-to-third-harmonic efficiency being close to 0.28. Our experimental results provide confirmation of expectations of the higher-order Kerr effect model.

  8. Generation of high-power tunable terahertz-radiation by nonrelativistic beam-echo harmonic effect

    SciTech Connect

    Gong Huarong; Xu Jin; Wei Yanyu; Gong Yubin; Travish, Gil; Feng Jinjun

    2013-01-15

    A new type of terahertz radiation source based on the nonrelativistic electron beam-wave interaction is proposed. Here, the beam echo harmonic effect is applied to a traveling wave tube like device. The scheme is configured as a combination of a frequency multiplier and amplifier with, for instance, W-band (millimeter wave) input signals and terahertz output power. A one-dimensional model of this device shows that a 10th order harmonic-wave can be generated while other harmonic waves are suppressed. The device only requires a readily available input source (W-band), and the output frequency can be tuned continuously over a wide band.

  9. Role of surface plasmon in second harmonic generation from gold nanorods

    SciTech Connect

    Hubert, C.; Billot, L.; Adam, P.-M.; Bachelot, R.; Royer, P.; Grand, J.; Gindre, D.; Dorkenoo, K. D.; Fort, A.

    2007-04-30

    The role of surface plasmon in second harmonic generation from arrays of gold nanorod particles excited by femtosecond laser pulses is investigated as a function of incident light polarization and irradiation wavelength. In addition to photoluminescence, a peak of second harmonic is observed and is found to depend on the polarization and wavelength of the fundamental frequency laser beam. In particular, the authors found similarities between extinction spectra of the nanoparticles and spectra of emmitted second harmonic. This behavior can be explained by resonant excitation of localized surface plasmon resonances.

  10. Relativistic second-harmonic generation of a laser from underdense plasmas

    SciTech Connect

    Singh, K.P.; Gupta, D.N.; Yadav, Sushila; Tripathi, V.K.

    2005-01-01

    A high intensity laser obliquely incident on a vacuum-plasma interface produces second-harmonic radiation in the reflected component. The efficiency of second-harmonic generation increases with the angle of incidence, up to critical angle of incidence (our model is not valid beyond critical angle of incidence). The efficiency also depends on electron density, showing a maximum at {omega}{sub p}{sup 2}/{omega}{sup 2} congruent with 0.7, where {omega}{sub p} and {omega} are relativistic plasma frequency and laser frequency, respectively. The efficiency of second-harmonic generation increases sharply with laser intensity in the nonrelativistic regime and saturates at higher intensities. The intensity of the second harmonic is proportional to square of the laser intensity at low pump laser intensities and tends to proportional to laser intensity in the strong relativistic regime.

  11. High-order harmonic generation using a high-repetition-rate turnkey laser

    SciTech Connect

    Lorek, E. Larsen, E. W.; Heyl, C. M.; Carlström, S.; Mauritsson, J.; Paleček, D.; Zigmantas, D.

    2014-12-15

    We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon, we achieve generation of photons with energies exceeding 90 eV (∼13 nm) at 20 kHz. We measure a photon flux of up to 4.4 × 10{sup 10} photons per second per harmonic in argon at 100 kHz. Many experiments employing high-order harmonics would benefit from higher repetition rates, and the user-friendly operation opens up for applications of coherent extreme ultra-violet pulses in new research areas.

  12. High-order harmonic generation using a high-repetition-rate turnkey laser.

    PubMed

    Lorek, E; Larsen, E W; Heyl, C M; Carlström, S; Paleček, D; Zigmantas, D; Mauritsson, J

    2014-12-01

    We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon, we achieve generation of photons with energies exceeding 90 eV (∼13 nm) at 20 kHz. We measure a photon flux of up to 4.4 × 10(10) photons per second per harmonic in argon at 100 kHz. Many experiments employing high-order harmonics would benefit from higher repetition rates, and the user-friendly operation opens up for applications of coherent extreme ultra-violet pulses in new research areas. PMID:25554271

  13. Coupled 2D Ag nano-resonator chains for enhanced and spatially tailored second harmonic generation.

    PubMed

    Centini, Marco; Benedetti, Alessio; Sibilia, Concita; Bertolotti, Mario

    2011-04-25

    We report results of second harmonic generation calculations performed on Silver coupled 2D-nanoresonators. Coupling is responsible for the creation of resonant modes that can be localized on small portions of the structure or distributed over the whole structure. Different field profiles can be obtained by varying the parameters of the input field (i.e. the wavelength). The second harmonic generation nonlinear process is enhanced by the excitation of coupled surface plasmon polaritons. The emitted field is strongly affected by the linear properties of the structure behaving as a nano antenna. We note that different configurations of the pump field lead to different second harmonic far-field emission patterns. Also, we show that the angular emission of the second harmonic field contains information about the spatial location of the pump field hot spots at different frequencies. Applications to a new class of nano sources for single molecule fluorescence and sensors are proposed.

  14. High harmonic generation in underdense plasmas by intense laser pulses with orbital angular momentum

    SciTech Connect

    Mendonça, J. T.; Vieira, J.

    2015-12-15

    We study high harmonic generation produced by twisted laser pulses, with orbital angular momentum in the relativistic regime, for pulse propagation in underdense plasma. We consider fast time scale processes associated with an ultra-short pulse, where the ion motion can be neglected. We use both analytical models and numerical simulations using a relativistic particle-in-cell code. The present description is valid for relativistic laser intensities, when the normalized field amplitude is much larger than one, a ≫ 1. We also discuss two distinct processes associated with linear and circular polarization. Using both analytical solutions and particle-in-cell simulations, we are able to show that, for laser pulses in a well defined Laguerre-Gauss mode, angular momentum conservation is observed during the process of harmonic generation. Intensity modulation of the harmonic spectrum is also verified, as imposed by the nonlinear time-scale for energy transfer between different harmonics.

  15. Using the self-filtering property of a femtosecond filament to improve second harmonic generation.

    PubMed

    Shwa, David; Eisenmann, Shmuel; Marcus, Gilad; Zigler, Arie

    2009-04-13

    In this paper we demonstrate the use of NIR femtosecond filament for improving the generation of second harmonic using a type I BBO crystal. Using this method the beam propagation factor (M(2)) of the second harmonic was improved significantly; which led to enhancement of the attainable SH intensity by up to two orders of magnitude. This method can be beneficial for applications demanding high intensities, small spot size or long interaction lengths.

  16. Low-order harmonic generation in nanosecond laser ablation plasmas of carbon containing materials

    NASA Astrophysics Data System (ADS)

    Lopez-Quintas, I.; Oujja, M.; Sanz, M.; Martín, M.; Ganeev, R. A.; Castillejo, M.

    2013-08-01

    In this work we report on a systematic study of the spatiotemporal behaviour of low-order harmonics generated in nanosecond laser ablation plasmas of carbon containing materials. Plasmas were generated from targets of graphite and boron carbide ablated with a nanosecond Q-switched Nd:YAG laser at 1064 nm. Low-order harmonics (3rd and 5th) of the fundamental wavelength of a ns Nd:YAG driving laser, propagating perpendicularly to the ablation laser at variable time delays, were observed. The temporal study of the low-order harmonics generated under vacuum and atmospheres of Kr and Xe, revealed the presence of two populations that contribute to the harmonic generation (HG) at different times. It was found that under vacuum only small species contribute to the HG process, whereas under buffer gas, heavier species, such as clusters and nanoparticles, contribute to the HG at longer times. Optical emission spectroscopy, time of flight mass spectrometry and characterization of deposits collected on-line on a nearby substrate provided additional information that complemented the results of the spatiotemporal study of the generated harmonics. This approach to ablation plume analysis allows elucidating the identity of the nonlinear emitters in laser ablation plasmas and facilitates the investigation of efficient, nanoparticle-enhanced, coherent short wavelength generation processes.

  17. Voyager high gain antenna calibration and pointing

    NASA Technical Reports Server (NTRS)

    Jahanshahi, M. H.

    1979-01-01

    A mathematical description of the data reduction technique used in analyzing Voyager calibration data is presented. To achieve the required telecommunication link performance, highly accurate pointing of the Voyager high gain antenna boresight relative to earth is necessary. To provide the optimum pointing, in-flight calibrations of the high gain antenna pointing mechanism are regularly made, and the design of the calibration and the antenna error models is delineated. It is shown that due to the use of wide angle sun sensors for celestial attitude control, the Voyager antenna error model differs from those of previous missions. Results of the in-flight calibrations and their implementation in improving the antenna pointing are also presented.

  18. Self Excitation and Harmonics in Wind Power Generation: Preprint

    SciTech Connect

    Muljadi, E.; Butterfield, C. P.; Romanowitz, H.; Yinger, R.

    2004-11-01

    Traditional wind turbines are equipped with induction generators. Induction generators are preferred because they are inexpensive, rugged, and require very little maintenance. Unfortunately, induction generators require reactive power from the grid to operate. Because reactive power varies with the output power, the terminal voltage at the generator may become too low to compensate the induction generator. The interactions among the wind turbine, the power network, and the capacitor compensation, are important aspects of wind generation. In this paper, we will show the interactions among the induction generator, capacitor compensation, power system network, and magnetic saturations and examine the cause of resonance conditions and self-excitation.

  19. Spectral modulation of third-harmonic generation by molecular alignment and preformed plasma

    NASA Astrophysics Data System (ADS)

    Li, Min; Li, An-Yuan; He, Bo-Qu; Yuan, Shuai; Zeng, He-Ping

    2016-08-01

    We demonstrate spectral modulation of third-harmonic generation from molecular alignment effects. The third harmonic spectrum is broadened or narrowed under different influences of cross-phase modulations originating from various molecular alignment revivals. Furthermore, the spectrum and spatial distribution of the generated third harmonic pulse change dramatically in the presence of a preformed plasma. Under the influence of a preformed plasma, a narrower third harmonic spectrum is observed, and the conical third-harmonic pulse increases while the axial part decreases. The investigation provides an effective method to modulate the spectral characteristic and spatial distribution of third-harmonic generation from intense femtosecond filament. Project supported by the National Key Scientific Instrument Project, China (Grant No. 2012YQ150092), the National Basic Research Program of China (Grant No. 2011CB808105), the National Natural Science Foundation of China (Grant No. 11434005), China Postdoctoral Science Foundation (Grant No. 2014M560348), the National Natural Science Foundation of China (Grant No. 11504237), and the Shanghai Municipal Science and Technology Commission, China (Grant No. 14JC1401600).

  20. Effects of electron relaxation on multiple harmonic generation from metal surfaces with femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Karatzas, N. E.; Georges, A. T.

    2006-11-01

    Calculations are presented for the first four (odd and even) harmonics of an 800 nm laser from a gold surface, with pulse widths ranging from 100 down to 14 fs. For peak laser intensities above 1 GW/cm 2 the harmonics are enhanced because of a partial depletion of the initial electron states. At 10 11 W/cm 2 of peak laser intensity the calculated conversion efficiency for 2nd-harmonic generation is 3 × 10 -9, while for the 5th-harmonic it is 10 -10. The generated harmonic pulses are broadened and delayed relative to the laser pulse because of the finite relaxation times of the excited electronic states. The finite electron relaxation times cause also the broadening of the autocorrelations of the laser pulses obtained from surface harmonic generation by two time-delayed identical pulses. Comparison with recent experimental results shows that the response time of an autocorrelator using nonlinear optical processes in a gold surface is shorter than the electron relaxation times. This seems to indicate that for laser pulses shorter than ˜30 fs, the fast nonresonant channel for multiphoton excitation via continuum-continuum transitions in metals becomes important as the resonant channel becomes slow (relative to the laser pulse) and less efficient.

  1. Surface area-dependent second harmonic generation from silver nanorods.

    PubMed

    Ngo, Hoang Minh; Luong, Thanh Tuyen; Ledoux-Rak, Isabelle

    2016-08-17

    The nonlinear optical (NLO) properties of metallic nanoparticles strongly depend on their size and shape. Metallic gold nanorods have already been widely investigated, but other noble metals could also be used for nanorod fabrication towards applications in photonics. Here we report on the synthesis and NLO characterization of silver nanorods (AgNRs) with controllable localized surface plasmon resonance. We have implemented an original, one-step and seedless synthesis method, based on a spontaneous particle growth technique in the presence of polyvinylpyrrolidone (PVP) as a capping agent. Colloidal solutions of AgNRs with various aspect ratios (5.0; 6.3; 7.5; 8.2 and 9.7) have been obtained and characterized using Harmonic light scattering (HLS) at 1064 nm, in order to investigate their quadratic NLO properties. From HLS experiments, we demonstrate that hyperpolarizability (β) values of AgNRs display a strong dependence on their surface area.

  2. Surface area-dependent second harmonic generation from silver nanorods.

    PubMed

    Ngo, Hoang Minh; Luong, Thanh Tuyen; Ledoux-Rak, Isabelle

    2016-08-17

    The nonlinear optical (NLO) properties of metallic nanoparticles strongly depend on their size and shape. Metallic gold nanorods have already been widely investigated, but other noble metals could also be used for nanorod fabrication towards applications in photonics. Here we report on the synthesis and NLO characterization of silver nanorods (AgNRs) with controllable localized surface plasmon resonance. We have implemented an original, one-step and seedless synthesis method, based on a spontaneous particle growth technique in the presence of polyvinylpyrrolidone (PVP) as a capping agent. Colloidal solutions of AgNRs with various aspect ratios (5.0; 6.3; 7.5; 8.2 and 9.7) have been obtained and characterized using Harmonic light scattering (HLS) at 1064 nm, in order to investigate their quadratic NLO properties. From HLS experiments, we demonstrate that hyperpolarizability (β) values of AgNRs display a strong dependence on their surface area. PMID:27498825

  3. High-order Harmonic Generation Driven by Sub-Cycle Shaped Laser Field

    NASA Astrophysics Data System (ADS)

    Zheng, Yinghui; Zeng, Zhinan; Wei, Pengfei; Miao, Jing; Li, Ruxin; Xu, Zhizhan

    High-order harmonic generation can be described by the semiclassical three-step model, in which an electron is freed, accelerated away from an atom or molecule by a strong oscillating laser field, and then, upon reversal of the field, careened back into its parent ion. The shaped laser field has been proved to be an effective tool to control the three-step process and consequently to achieve the high intensity harmonic generation or an isolated attosecond pulse generation by changing the relative phase, intensity ratio, polarization, etc, between the pulses of shaped laser field. High-order harmonic and attosecond pulse generation driven by a shaped laser field synthesized with two or three laser pulses of controlled related phase are reviewed.

  4. Imaging the bipolarity of myosin filaments with Interferometric Second Harmonic Generation microscopy

    PubMed Central

    Rivard, Maxime; Couture, Charles-André; Miri, Amir K.; Laliberté, Mathieu; Bertrand-Grenier, Antony; Mongeau, Luc; Légaré, François

    2013-01-01

    We report that combining interferometry with Second Harmonic Generation (SHG) microscopy provides valuable information about the relative orientation of noncentrosymmetric structures composing tissues. This is confirmed through the imaging of rat medial gastrocnemius muscle. The inteferometric Second Harmonic Generation (ISHG) images reveal that each side of the myosin filaments composing the A band of the sarcomere generates π phase shifted SHG signal which implies that the myosin proteins at each end of the filaments are oriented in opposite directions. This highlights the bipolar structural organization of the myosin filaments and shows that muscles can be considered as a periodically poled biological structure. PMID:24156065

  5. Structural light focusing phenomenon and enhanced second harmonic generation in NaNO2-infiltrated opal photonic crystal

    NASA Astrophysics Data System (ADS)

    Zaytsev, Kirill I.; Katyba, Gleb M.; Yakovlev, Egor V.; Aliev, Ismail N.; Khorokhorov, Alexey M.; Yurchenko, Stanislav O.

    2015-01-01

    We report new experimental results on enhanced second harmonic generation using a structural light focusing phenomenon in photonic crystals (PCs). We use opal-based PC, infiltrated with NaNO2 and pumped with femtosecond laser pulses at various incidence angles, in order to examine the dependence of second harmonic generation efficiency on the pumping wavelength location toward the PC band-gap. We demonstrate one order enhancement of second harmonic generation in case of PC band-gap pumping in comparison to non-band- gap pumping. Second harmonic generation is performed in reflection mode with the maximum of generation in the direction of mirror reflection. We demonstrate that the spectrum of second harmonic does not narrow with the quasi-phase matching condition in case of band-gap generation, and second harmonic spectrum corresponding to non-band-gap generation undergoes 1.5 times narrowing due to the quasi-phase matching.

  6. Acoustic harmonic generation from fatigue-generated dislocation substructures in copper single crystals

    NASA Astrophysics Data System (ADS)

    Apple, T. M.; Cantrell, J. H.; Amaro, C. M.; Mayer, C. R.; Yost, W. T.; Agnew, S. R.; Howe, J. M.

    2013-07-01

    Dislocations generated during cyclic loading of metals self-organize into substructures that produce substantial changes in the nonlinear response. The nonlinearity is quantified by the material nonlinearity parameter ? extracted from acoustic harmonic generation measurements. Measurements of ? on copper single crystals oriented for single-slip ([1 2 3] loading axis) and fatigued in plastic strain control are compared to calculations of ? obtained from the Cantrell model for which measured values of model parameters associated with the substructures are required. Transmission electron microscopy measurements of the volume fractions of veins and persistent slip bands, dislocation loop lengths, dipole heights and the densities of primary and secondary dislocations in the fatigue-generated substructures are obtained for input into the model calculations. The model predictions agree with the values observed experimentally. In particular, the experimental data show an increase in ? proportional to ? where ? is the cumulative plastic strain and m is 0.7 and 0.4, respectively, for acoustic wave propagation along the ? and ? crystal axes. Such dependence is consistent with the Cantrell model and at variance with models, based on assumed variations in the third-order elastic constants, which predict an exponential dependence on ? .

  7. Dependence of high-order-harmonic generation on dipole moment in Si O2 crystals

    NASA Astrophysics Data System (ADS)

    Yu, Chao; Zhang, Xirui; Jiang, Shicheng; Cao, Xu; Yuan, Guanglu; Wu, Tong; Bai, Lihua; Lu, Ruifeng

    2016-07-01

    High-order-harmonic generation in α-quartz Si O2 is theoretically investigated under a strong laser field by solving the extended semiconductor Bloch equations. The accurate band structures as well as dipole moments between different bands are obtained from state-of-the-art first-principles calculations. We find that the shapes of k -space-dependent dipole moments play an important role in harmonic generation. The calculated results show that harmonic conversion efficiency is significantly enhanced and the cutoff energy is distinctly increased when the dipole moments change greatly along a valley in the k direction in the solid. Based on that dependence on the dipole moment, we also show that symmetry groups greatly affect the harmonic spectra from the solid materials. Moreover, a two-color synthesized field is used to achieve a supercontinuum harmonic spectrum near the cutoff region, and isolated attosecond pulses can be obtained directly by filtering out the harmonic radiation. We hope the contribution presented in this work provides a useful reference for future studies on laser-crystal interactions.

  8. Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation

    PubMed Central

    Ferré, A.; Boguslavskiy, A. E.; Dagan, M.; Blanchet, V.; Bruner, B. D.; Burgy, F.; Camper, A.; Descamps, D.; Fabre, B.; Fedorov, N.; Gaudin, J.; Geoffroy, G.; Mikosch, J.; Patchkovskii, S.; Petit, S.; Ruchon, T.; Soifer, H.; Staedter, D.; Wilkinson, I.; Stolow, A.; Dudovich, N.; Mairesse, Y.

    2015-01-01

    High-order harmonic generation in polyatomic molecules generally involves multiple channels of ionization. Their relative contribution can be strongly influenced by the presence of resonances, whose assignment remains a major challenge for high-harmonic spectroscopy. Here we present a multi-modal approach for the investigation of unaligned polyatomic molecules, using SF6 as an example. We combine methods from extreme-ultraviolet spectroscopy, above-threshold ionization and attosecond metrology. Fragment-resolved above-threshold ionization measurements reveal that strong-field ionization opens at least three channels. A shape resonance in one of them is found to dominate the signal in the 20–26 eV range. This resonance induces a phase jump in the harmonic emission, a switch in the polarization state and different dynamical responses to molecular vibrations. This study demonstrates a method for extending high-harmonic spectroscopy to polyatomic molecules, where complex attosecond dynamics are expected. PMID:25608712

  9. Optimization of multi-color laser waveform for high-order harmonic generation

    NASA Astrophysics Data System (ADS)

    Jin, Cheng; Lin, C. D.

    2016-09-01

    With the development of laser technologies, multi-color light-field synthesis with complete amplitude and phase control would make it possible to generate arbitrary optical waveforms. A practical optimization algorithm is needed to generate such a waveform in order to control strong-field processes. We review some recent theoretical works of the optimization of amplitudes and phases of multi-color lasers to modify the single-atom high-order harmonic generation based on genetic algorithm. By choosing different fitness criteria, we demonstrate that: (i) harmonic yields can be enhanced by 10 to 100 times, (ii) harmonic cutoff energy can be substantially extended, (iii) specific harmonic orders can be selectively enhanced, and (iv) single attosecond pulses can be efficiently generated. The possibility of optimizing macroscopic conditions for the improved phase matching and low divergence of high harmonics is also discussed. The waveform control and optimization are expected to be new drivers for the next wave of breakthrough in the strong-field physics in the coming years. Project supported by the Fundamental Research Funds for the Central Universities of China (Grant No. 30916011207), Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U. S. Department of Energy (Grant No. DE-FG02-86ER13491), and Air Force Office of Scientific Research, USA (Grant No. FA9550-14-1-0255).

  10. High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis

    SciTech Connect

    Madsen, C. B.; Abu-samha, M.; Madsen, L. B.

    2010-04-15

    We present a generic approach for treating the effect of nuclear motion in high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the electronic part using the Lewenstein model and nuclear motion enters as a nuclear correlation function. We express the nuclear correlation function in terms of Franck-Condon factors, which allows us to decompose nuclear motion into modes and identify the modes that are dominant in the high-order harmonic generation process. We show results for the isotopes CH{sub 4} and CD{sub 4} and thereby provide direct theoretical support for a recent experiment [S. Baker et al., Science 312, 424 (2006)] that uses high-order harmonic generation to probe the ultrafast structural nuclear rearrangement of ionized methane.

  11. Harmonic signal generation and frequency upconversion using selective sideband Brillouin amplification in single-mode fiber.

    PubMed

    Lee, Kwang-Hyun; Choi, Woo-Young

    2007-06-15

    Harmonic signal generation and frequency upconversion at millimeter-wave bands are experimentally demonstrated by using selective sideband Brillouin amplification induced by stimulated Brillouin scattering in a single-mode fiber. The harmonic signals and frequency upconverted signals are simultaneously generated by the beating of optical sidebands, one of which is Brillouin amplified. By using this method, we successfully demonstrate generation of third-harmonic millimeter waves at 32.55 GHz with f(LO) of 10.85 GHz and upconversion of 10 Mbps quadrature-shift keyed data at f(IF) of 1.55 GHz into a 30 GHz band with more than 17 dB RF power gain.

  12. Spherical harmonic analysis of a synoptic climatology generated with a global general circulation model

    NASA Technical Reports Server (NTRS)

    Christidis, Z. D.; Spar, J.

    1980-01-01

    Spherical harmonic analysis was used to analyze the observed climatological (C) fields of temperature at 850 mb, geopotential height at 500 mb, and sea level pressure. The spherical harmonic method was also applied to the corresponding "model climatological" fields (M) generated by a general circulation model, the "GISS climate model." The climate model was initialized with observed data for the first of December 1976 at 00. GMT and allowed to generate five years of meteorological history. Monthly means of the above fields for the five years were computed and subjected to spherical harmonic analysis. It was found from the comparison of the spectral components of both sets, M and C, that the climate model generated reasonable 500 mb geopotential heights. The model temperature field at 850 mb exhibited a generally correct structure. However, the meridional temperature gradient was overestimated and overheating of the continents was observed in summer.

  13. Enhanced second-harmonic-generation detection of collagen by means of optical wavefront shaping

    NASA Astrophysics Data System (ADS)

    Thompson, Jonathan V.; Throckmorton, Graham A.; Hokr, Brett H.; Yakovlev, Vladislav V.

    2016-03-01

    Second-harmonic generation (SHG) has proven to be an effective method to both image and detect structural variations in fibrillar collagen. The ability to detect these differences is especially useful in studying diseases like cancer and fibrosis.1 SHG techniques have historically been limited by their ability to penetrate and image through strongly scattering tissues. Recently, optical wavefront shaping has enabled light to be focused through highly scattering media such as biological tissue.2-4 This technology also enables us to examine the dependence of second harmonic generation on the spatial phase of the pump laser. Here, we demonstrate that wavefront shaping can be used to enhance the generation of second harmonic light from collagen fibrils even when scattering is low or non-existent.

  14. Macroscopic manipulation of high-order-harmonic generation through bound-state coherent control.

    PubMed

    Hadas, Itai; Bahabad, Alon

    2014-12-19

    We propose a paradigm for macroscopic control of high-order harmonic generation by modulating the bound-state population of the medium atoms. A unique result of this scheme is that apart from regular spatial quasi-phase-matching (QPM), also purely temporal QPM of the emitted radiation can be established. Our simulations demonstrate temporal QPM by inducing homogenous Rabi oscillations in the medium and also spatial QPM by creating a grating of population inversion using the process of rapid adiabatic passage. In the simulations a scaled version of high-order harmonic generation is used: a far off-resonance 2.6  μm source generates UV-visible high-order harmonics from alkali-metal-atom vapor, while a resonant near IR source is used to coherently control the medium.

  15. High-order harmonic generation from Rydberg atoms in inhomogeneous fields.

    PubMed

    Wang, Zhe; He, Lixin; Luo, Jianghua; Lan, Pengfei; Lu, Peixiang

    2014-10-20

    We theoretically investigate the high-order harmonic generation (HHG) from Rydberg atoms considering the spatial inhomogeneity of the driving field. It is found that in the inhomogeneous field, the effect of the cutoff extension in the harmonic spectrum from Rydberg atoms can be extended to multi-cycle regime, while in the homogeneous field case, the extension of the harmonic cutoff is limited to the few-cycle regime (less than two optical cycles). The underlying physics of the cutoff extension from Rydberg atoms in the inhomogeneous field is analyzed based on the classical and quantum-mechanical models. Furthermore, by optimizing the field inhomogeneity, the electron dynamics can be well controlled to generate a smooth supercontinuum in the extended spectral region. This can support the efficient generation of isolated attosecond pulses in Rydberg atoms from multi-cycle laser fields.

  16. Galileo spacecraft high gain antenna offset calibration

    NASA Technical Reports Server (NTRS)

    Hayati, S. A.

    1982-01-01

    A mathematical model for the estimation of the dual-spin Galileo spacecraft high gain antenna misalignment is developed. The feasibility of the proposed technique is investigated by means of a simulation study. In-flight parameter estimation requires the development of a stochastic model of the spacecraft rotational biases and the earth-received signal strength measurements. The signal strength measurements for X-band frequency are used as observations to estimate the rotational biases and their corresponding uncertainties. The simulation study shows that the initial ground measured uncertainties of .6 mrad can be reduced by a factor of ten.

  17. Three-dimensional nanostructures as highly efficient generators of second harmonic light.

    PubMed

    Zhang, Yu; Grady, Nathaniel K; Ayala-Orozco, Ciceron; Halas, Naomi J

    2011-12-14

    Plasmonic nanostructures enable the generation of large electromagnetic fields confined to small volumes, potentially providing a route for the development of nanoengineered nonlinear optical media. A metal-capped hemispherical nanoparticle, also known as a nanocup, generates second harmonic light with increasing intensity as the angle between the incident fundamental beam and the nanocup symmetry axis is increased. Nanoparticle orientation also modifies the emission direction of the second harmonic light. With conversion efficiencies similar to those of inorganic SHG crystals, these structures provide a promising approach for the design and fabrication of stable, synthetic second-order nonlinear optical materials tailored for specific wavelengths.

  18. Quasi-phase-matched backward second-harmonic generation by complementary media in nonlinear metamaterials.

    PubMed

    Quan, Li; Liu, Xiaozhou; Gong, Xiufen

    2012-10-01

    High efficiency of the second-harmonic and sum-frequency generation can be obtained in optical superlattice by using the conventional quasi-phase-matched (QPM) method. Although this trick can be played on the acoustic wave, the media with negative nonlinear parameters are not common in acoustics. Furthermore, the QPM method used in acoustic metamaterials has been less studied. In this work, a protocol is provided to realize the QPM method by using nonlinear complementary media in acoustic metamaterials in order to obtain large backward second-harmonic generation. Compared with the conventional method, the method gains a broader bandwidth and can be used in both acoustic and electromagnetic waves.

  19. High-order harmonic generation at a repetition rate of 100 kHz

    SciTech Connect

    Lindner, F.; Stremme, W.; Schaetzel, M. G.; Grasbon, F.; Paulus, G. G.; Walther, H.; Hartmann, R.; Strueder, L.

    2003-07-01

    We report high-order harmonic generation (HHG) in rare gases using a femtosecond laser system with a very high repetition rate (100 kHz) and low pulse energy (7 {mu}J). To our knowledge, this is the highest repetition rate reported to date for HHG. The tight focusing geometry required to reach sufficiently high intensities implies low efficiency of the process. Harmonics up to the 45th order are nevertheless generated and detected. We show evidence of clear separation and selection of quantum trajectories by moving the gas jet with respect to the focus, in agreement with the theoretical predictions of the semiclassical model of HHG.

  20. Multielectron Correlation in High-Harmonic Generation: A 2D Model Analysis

    SciTech Connect

    Sukiasyan, Suren; McDonald, Chris; Destefani, Carlos; Brabec, Thomas; Ivanov, Misha Yu.

    2009-06-05

    We analyze the role of multielectron dynamics in high-harmonic generation spectroscopy, using an example of a two-electron system. We identify and systematically quantify the importance of correlation and exchange effects. One of the main sources for correlation is identified to be the polarization of the ion by the recombining continuum electron. This effect, which plays an important qualitative and quantitative role, seriously undermines the validity of the standard approaches to high-harmonic generation, which ignore the contribution of excited ionic states to the radiative recombination of the continuum electron.

  1. Cavity-Enhanced High-Harmonic Generation with Spatially Tailored Driving Fields

    NASA Astrophysics Data System (ADS)

    Pupeza, I.; Högner, M.; Weitenberg, J.; Holzberger, S.; Esser, D.; Eidam, T.; Limpert, J.; Tünnermann, A.; Fill, E.; Yakovlev, V. S.

    2014-03-01

    We theoretically and experimentally investigate high-harmonic generation in a 78-MHz enhancement cavity with a transverse mode having on-axis intensity maxima at the focus and minima at an opening in the following mirror. We find that the conversion efficiency is comparable to that achievable with a Gaussian mode, whereas the output coupling efficiency can be significantly improved over any other demonstrated technique. This approach offers additional power scaling advantages and additional degrees of freedom in shaping the harmonic emission, paving the way to high-power extreme-ultraviolet frequency combs and the generation of multi-MHz repetition-rate-isolated attosecond pulses.

  2. Life Cycle GHG Emissions from Conventional Natural Gas Power Generation: Systematic Review and Harmonization (Presentation)

    SciTech Connect

    Heath, G.; O'Donoughue, P.; Whitaker, M.

    2012-12-01

    This research provides a systematic review and harmonization of the life cycle assessment (LCA) literature of electricity generated from conventionally produced natural gas. We focus on estimates of greenhouse gases (GHGs) emitted in the life cycle of electricity generation from conventionally produced natural gas in combustion turbines (NGCT) and combined-cycle (NGCC) systems. A process we term "harmonization" was employed to align several common system performance parameters and assumptions to better allow for cross-study comparisons, with the goal of clarifying central tendency and reducing variability in estimates of life cycle GHG emissions. This presentation summarizes preliminary results.

  3. Huge enhancement of backward second-harmonic generation with slow light in photonic crystals

    SciTech Connect

    Iliew, Rumen; Etrich, Christoph; Pertsch, Thomas; Kivshar, Yuri S.

    2010-02-15

    We study theoretically forward and backward second-harmonic generation in a two-dimensional photonic crystal structure made of lithium niobate. The aim of this article is twofold: First, we propose a reliable modal algorithm for describing the light propagation taking into account the vectorial character of the interacting fields as well as the tensorial character of the nonlinearity and verify it by means of the nonlinear finite-difference time-domain method. Second, we propose a photonic crystal where we obtain a giant efficiency increase for backward second-harmonic generation with slow light.

  4. Second harmonic generation in photonic crystal cavities in (111)-oriented GaAs

    SciTech Connect

    Buckley, Sonia Radulaski, Marina; Vučković, Jelena; Biermann, Klaus

    2013-11-18

    We demonstrate second harmonic generation at telecommunications wavelengths in photonic crystal cavities in (111)-oriented GaAs. We fabricate 30 photonic crystal structures in both (111)- and (100)-oriented GaAs and observe an increase in generated second harmonic power in the (111) orientation, with the mean power increased by a factor of 3, although there is a large scatter in the measured values. We discuss possible reasons for this increase, in particular, the reduced two photon absorption for transverse electric modes in (111) orientation, as well as a potential increase due to improved mode overlap.

  5. Quadrupole second harmonic generation and sum-frequency generation in ZnO quantum dots

    SciTech Connect

    Maikhuri, Deepti; Purohit, S. P. Mathur, K. C.

    2015-04-15

    The second harmonic generation (SHG) and the sum frequency generation (SFG) processes are investigated in the conduction band states of the singly charged ZnO quantum dot (QD) embedded in the HfO{sub 2}, and the AlN matrices. With two optical fields of frequency ω{sub p} and ω{sub q} incident on the dot, we study the variation with frequency of the second order nonlinear polarization resulting in SHG and SFG, through the electric dipole and the electric quadrupole interactions of the pump fields with the electron in the dot. We obtain enhanced value of the second order nonlinear susceptibility in the dot compared to the bulk. The effective mass approximation with the finite confining barrier is used for obtaining the energy and wavefunctions of the quantized confined states of the electron in the conduction band of the dot. Our results show that both the SHG and SFG processes depend on the dot size, the surrounding matrix and the polarization states of the pump beams.

  6. High-Gain High-Field Fusion Plasma.

    PubMed

    Li, Ge

    2015-01-01

    A Faraday wheel (FW)-an electric generator of constant electrical polarity that produces huge currents-could be implemented in an existing tokamak to study high-gain high-field (HGHF) fusion plasma, such as the Experimental Advanced Superconducting Tokamak (EAST). HGHF plasma can be realized in EAST by updating its pulsed-power system to compress plasma in two steps by induction fields; high gains of the Lawson trinity parameter and fusion power are both predicted by formulating the HGHF plasma. Both gain rates are faster than the decrease rate of the plasma volume. The formulation is checked by earlier ATC tests. Good agreement between theory and tests indicates that scaling to over 10 T at EAST may be possible by two-step compressions with a compression ratio of the minor radius of up to 3. These results point to a quick new path of fusion plasma study, i.e., simulating the Sun by EAST. PMID:26507314

  7. High-Gain High-Field Fusion Plasma

    NASA Astrophysics Data System (ADS)

    Li, Ge

    2015-10-01

    A Faraday wheel (FW)—an electric generator of constant electrical polarity that produces huge currents—could be implemented in an existing tokamak to study high-gain high-field (HGHF) fusion plasma, such as the Experimental Advanced Superconducting Tokamak (EAST). HGHF plasma can be realized in EAST by updating its pulsed-power system to compress plasma in two steps by induction fields; high gains of the Lawson trinity parameter and fusion power are both predicted by formulating the HGHF plasma. Both gain rates are faster than the decrease rate of the plasma volume. The formulation is checked by earlier ATC tests. Good agreement between theory and tests indicates that scaling to over 10 T at EAST may be possible by two-step compressions with a compression ratio of the minor radius of up to 3. These results point to a quick new path of fusion plasma study, i.e., simulating the Sun by EAST.

  8. Free-electron laser harmonic generation in an electromagnetic-wave wiggler and ion channel guiding

    SciTech Connect

    Mehdian, H.; Hasanbeigi, A.; Jafari, S.

    2010-02-15

    A theoretical study of electron trajectories, harmonic generation, and gain in a free-electron laser (FEL) with a linearly polarized electromagnetic-wave wiggler is presented for axial injection of electron beam. The relativistic equation of motion for a single electron has been derived and solved numerically. It is found that the trajectories consist of two regimes. The stability of these regimes has been investigated. The results show that the trajectories are stable except for some parts of the regime one. The effects of interaction on the transverse velocity of the electron are a superposition of two oscillation terms, one at the wiggler frequency and the other at the betatron ion-channel frequency. A detailed analysis of the gain equation in the low-gain-per-pass limit has been employed to investigate FEL operation in higher harmonics generation. The possibility of wave amplification at both wiggler frequency and betatron ion-channel frequency for their odd harmonics has been illustrated.

  9. Effect of localized microstructural evolution on higher harmonic generation of guided wave modes

    NASA Astrophysics Data System (ADS)

    Choi, Gloria; Liu, Yang; Yao, Xiaochu; Lissenden, Cliff J.

    2015-03-01

    Higher harmonic generation of ultrasonic waves has the potential to be used to detect precursors to macroscale damage of phenomenon like fatigue due to microstructural evolution contributing to nonlinear material behavior. Aluminum plates having various plastic zone sizes were plastically deformed to different levels. The fundamental shear horizontal mode was then generated in the plate samples via a magnetostrictive transducer. After propagating through the plastic zone the primary wave mode (SH0) and its third harmonic (sh0) were received by a second transducer. Results of a parallel numerical study using the S1-s2 Lamb mode pair, where sensitivity to changes in third order elastic constants were investigated, are described within the context of the experimental results. Specimens used within both studies are geometrically similar and have double edge notches for dog bone samples that introduce localized plastic deformation. Through both studies, the size of the plastic zone with respect to the propagation distance and damage intensity influence the higher harmonics.

  10. Silencing and enhancement of second-harmonic generation in optical gap antennas.

    PubMed

    Berthelot, Johann; Bachelier, Guillaume; Song, Mingxia; Rai, Padmnabh; Colas des Francs, Gérard; Dereux, Alain; Bouhelier, Alexandre

    2012-05-01

    Amplifying local electromagnetic fields by engineering optical interactions between individual constituents of an optical antenna is considered fundamental for efficient nonlinear wavelength conversion in nanometer-scale devices. In contrast to this general statement we show that high field enhancement does not necessarily lead to an optimized nonlinear activity. In particular, we demonstrate that second-harmonic responses generated at strongly interacting optical gap antennas can be significantly suppressed. Numerical simulations are confirming silencing of second-harmonic in these coupled systems despite the existence of local field amplification. We then propose a simple approach to restore and amplify the second-harmonic signal by changing the manner in which electrically-connected optical antennas are interacting in the charge-transfer plasmon regime. Our observations provide critical design rules for realizing optimal structures that are essential for a broad variety of nonlinear surface-enhanced characterizations and for realizing the next generation of electrically-driven optical antennas.

  11. High-speed measurement of rotational anisotropy nonlinear optical harmonic generation using position-sensitive detection.

    PubMed

    Harter, J W; Niu, L; Woss, A J; Hsieh, D

    2015-10-15

    We present a method of performing high-speed rotational anisotropy nonlinear optical harmonic generation experiments at rotational frequencies of several hertz by projecting the harmonic light reflected at different angles from a sample onto a stationary position-sensitive detector. The high rotational speed of the technique, 10(3) to 10(4) times larger than existing methods, permits precise measurements of the crystallographic and electronic symmetries of samples by averaging over low frequency laser-power, beam-pointing, and pulse-width fluctuations. We demonstrate the sensitivity of our technique by resolving the bulk fourfold rotational symmetry of GaAs about its [001] axis using second-harmonic generation. PMID:26469591

  12. Role of ellipticity in high-order harmonic generation by homonuclear diatomic molecules

    SciTech Connect

    Odzak, S.; Milosevic, D. B.

    2010-08-15

    We present a theory of high-order harmonic generation by diatomic molecules exposed to an elliptically polarized laser field. This theory is based on the molecular strong-field approximation with the laser-field-dressed initial bound state and the undressed final state. The interference minima, observed for linear polarization, are blurred with the increase of the laser-field ellipticity. The nth harmonic emission rate has contributions of the components of the T-matrix element in the direction of the laser-field polarization and in the direction perpendicular to it. We analyze the destructive interference condition for this perpendicular component. Taking into account that the aligned molecules are an anisotropic medium for high-harmonic generation, we introduce elliptic dichroism as a measure of this anisotropy and discuss possibilities of its use for determining the molecular structure.

  13. Generation of the numerator = 2 rational harmonic mode-locked pulses in fiber ring lasers

    NASA Astrophysics Data System (ADS)

    Wang, Pinghe; Zhan, Li; Ye, Qinghao; Xia, Yuxing

    2004-09-01

    In conventional rational harmonic mode-locking, optical pulse trains with the repetition rate of (pn+1)f_(c) are generated when the modulation frequency of the in-cavity modulator is set at f_(m)=(n+1/p)f_(c), where n and p are both integers, f_(c) is the fundamental cavity frequency. In this paper, we report that rational harmonic mode locking phenomenon takes place in the fiber lasers when the modulation frequency is set at f_(m)=(n+2/p)f_(c). The pulse generations are experimentally demonstrated when the numerator of the rational corresponds to 2 in 5th and 7th order rational harmonic mode-locking.

  14. Sensitivity of Second Harmonic Generation from Styryl Dyes to Transmembrane Potential

    PubMed Central

    Millard, Andrew C.; Jin, Lei; Wei, Mei-de; Wuskell, Joseph P.; Lewis, Aaron; Loew, Leslie M.

    2004-01-01

    In this article we present results from the simultaneous nonlinear (second harmonic generation and two-photon excitation fluorescence) imaging and voltage clamping of living cells. Specifically, we determine the sensitivity to transmembrane potential of second harmonic generation by ANEP-chromophore styryl dyes as a function of excitation wavelength and dye structure. We have measured second harmonic sensitivities of up to 43% per 100 mV, more than a factor of four better than the nominal voltage sensitivity of the dyes under “one-photon” fluorescence. We find a dependence of voltage sensitivity on excitation wavelength that is consistent with a two-photon resonance, and there is a significant dependence of voltage sensitivity on the structure of the nonchromophore portion of the dyes. PMID:14747351

  15. Nonlinear absorption and harmonic generation of laser in a gas with anharmonic clusters

    SciTech Connect

    Kumar, Manoj; Tripathi, V. K.

    2013-02-15

    The nonlinear absorption and harmonic generation of intense short pulse laser in a gas embedded with anharmonic clusters are investigated theoretically. When the laser induced excursion of cluster electrons becomes comparable to cluster radius, the restoration force on electrons no longer remains linearly proportional to the excursion. As a consequence, the plasmon resonance is broadened, leading to broadband laser absorption. It also leads to second and third harmonic generations, at much higher level than the one due to ponderomotive nonlinearity. The harmonic yield is resonantly enhanced at the plasmon resonance {omega}={omega}{sub pe}/{radical}(3), where {omega} is the frequency of the laser and {omega}{sub pe} is the plasma frequency of cluster electrons.

  16. Characteristics of second harmonic generation of Lamb waves in nonlinear elastic plates.

    PubMed

    Müller, Martin F; Kim, Jin-Yeon; Qu, Jianmin; Jacobs, Laurence J

    2010-04-01

    This paper investigates the characteristics of the second harmonic generation of Lamb waves in a plate with quadratic nonlinearity. Analytical asymptotic solutions to Lamb waves are first obtained through the use of a perturbation method. Then, based on a careful analysis of these asymptotic solutions, it is shown that the cross-modal generation of a symmetric second harmonic mode by an antisymmetric primary mode is possible. These solutions also demonstrate that modes showing internal resonance-nonzero power flux to the second harmonic mode, plus phase velocity matching-are most useful for measurements. In addition, when using finite wave packets, which is the case in most experimental measurements, group velocity matching is required for a cumulative increase in the second harmonic amplitude with propagation distance. Finally, five mode types (which are independent of material properties) that satisfy all three requirements for this cumulative increase in second harmonic amplitude-nonzero power flux, plus phase and group velocity matching-are identified. These results are important for the development of an experimental procedure to measure material nonlinearity with Lamb waves.

  17. Harmonic generation at high field strengths - Frequency shifts and saturation phenomena. [optical mixing technique

    NASA Technical Reports Server (NTRS)

    Stappaerts, E. A.

    1975-01-01

    Optical harmonic generation and mixing in the gas phase has been proposed as a technique for the generation of coherent radiation in the vacuum ultraviolet and soft X-ray spectral region. At the high field strengths required by these processes the interaction between atoms and the electromagnetic field shows intensity-dependent resonances. In this paper we modify harmonic generation theory to include the effect of these frequency shifts. Closed-form expressions for generated dipole moment, absorption probability, and coherence length are presented. The most important consequences of frequency shifts on resonantly enhanced processes are that the pump laser must be tuned away from the small-field resonance frequency, that the conversion efficiency may saturate, and that the dispersion of the medium may change sign. As an example, the generation of 198-A radiation by a five-photon mixing process in Li(+) is considered.

  18. Using the third state of matter: high harmonic generation from liquid targets

    NASA Astrophysics Data System (ADS)

    Heissler, P.; Lugovoy, E.; Hörlein, R.; Waldecker, L.; Wenz, J.; Heigoldt, M.; Khrennikov, K.; Karsch, S.; Krausz, F.; Abel, B.; Tsakiris, G. D.

    2014-11-01

    High harmonic generation on solid and gaseous targets has been proven to be a powerful platform for the generation of attosecond pulses. Here we demonstrate a novel technique for the XUV generation on a smooth liquid surface target in vacuum, which circumvents the problem of low repetition rate and limited shot numbers associated with solid targets, while it maintains some of its merits. We employed atomically smooth, continuous liquid jets of water, aqueous salt solutions and ethanol that allow uninterrupted high harmonic generation due to the coherent wake emission mechanism for over 8 h. It has been found that the mechanism of plasma generation is very similar to that for smooth solid target surfaces. The vapor pressure around the liquid target in our setup has been found to be very low such that the presence of the gas phase around the liquid jet could be neglected.

  19. Laser-Induced Periodical Structures Fabrication for Third Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Voytova, T. A.; Makarov, S. V.; Tsypkin, A. N.; Milichko, V. A.; Mukhin, I. S.; Yulin, A. V.; Putilin, S. E.; Baranov, M. A.; Krasnok, A. E.; Belov, P. A.

    2016-08-01

    We propose a novel strategy for self-adjusted fabrication of large-scale array of resonant silicon nanoparticles (metasurface) on a thin silicon film. The self-adjusting mechanism is based on the effect of resonant nanogratings formation under intense multishot femtosecond irradiation of a thin silicon film. The resulting metasurfaces allow for generation of ultraviolet laser pulses at a wavelength of 270 nm with conversion efficiency up to 10-6 and high peak (≈100 kW/sm2) and average power (≈1.5 μW). Such high peak power from ultrathin metasurface makes the generated UV pulses applicable in a wide range of applications: precise nanolithography, ultrafast photoexcitation etc.

  20. Probing Ferroelectric Domain Engineering in BiFeO3 Thin Films by Second Harmonic Generation.

    PubMed

    Trassin, Morgan; Luca, Gabriele De; Manz, Sebastian; Fiebig, Manfred

    2015-09-01

    An optical probe of the ferroelectric domain distribution and manipulation in BiFeO3 thin films is reported using optical second harmonic generation. A unique relation between the domain distribution and its integral symmetry is established. The ferroelectric signature is even resolved when the film is covered by a top electrode. The effect of voltage-induced ferroelectric switching is imaged.

  1. Continuous-variable Einstein-Podolsky-Rosen paradox with traveling-wave second-harmonic generation

    SciTech Connect

    Olsen, M.K.

    2004-09-01

    The Einstein-Podolsky-Rosen paradox and quantum entanglement are at the heart of quantum mechanics. Here we show that single-pass traveling-wave second-harmonic generation can be used to demonstrate both entanglement and the paradox with continuous variables that are analogous to the position and momentum of the original proposal.

  2. Real-time observation of interfering crystal electrons in high-harmonic generation.

    PubMed

    Hohenleutner, M; Langer, F; Schubert, O; Knorr, M; Huttner, U; Koch, S W; Kira, M; Huber, R

    2015-07-30

    Acceleration and collision of particles has been a key strategy for exploring the texture of matter. Strong light waves can control and recollide electronic wavepackets, generating high-harmonic radiation that encodes the structure and dynamics of atoms and molecules and lays the foundations of attosecond science. The recent discovery of high-harmonic generation in bulk solids combines the idea of ultrafast acceleration with complex condensed matter systems, and provides hope for compact solid-state attosecond sources and electronics at optical frequencies. Yet the underlying quantum motion has not so far been observable in real time. Here we study high-harmonic generation in a bulk solid directly in the time domain, and reveal a new kind of strong-field excitation in the crystal. Unlike established atomic sources, our solid emits high-harmonic radiation as a sequence of subcycle bursts that coincide temporally with the field crests of one polarity of the driving terahertz waveform. We show that these features are characteristic of a non-perturbative quantum interference process that involves electrons from multiple valence bands. These results identify key mechanisms for future solid-state attosecond sources and next-generation light-wave electronics. The new quantum interference process justifies the hope for all-optical band-structure reconstruction and lays the foundation for possible quantum logic operations at optical clock rates.

  3. Enhanced second harmonic generation by photonic-plasmonic Fano-type coupling in nanoplasmonic arrays.

    PubMed

    Walsh, Gary F; Dal Negro, Luca

    2013-07-10

    In this communication, we systematically investigate the effects of Fano-type coupling between long-range photonic resonances and localized surface plasmons on the second harmonic generation from periodic arrays of Au nanoparticles arranged in monomer and dimer geometries. Specifically, by scanning the wavelength of an ultrafast tunable pump laser over a large range, we measure the second harmonic excitation spectra of these arrays and demonstrate their tunability with particle size and separation. Moreover, through a comparison with linear optical transmission spectra, which feature asymmetric Fano-type lineshapes, we demonstrate that the second harmonic generation is enhanced when coupled photonic-plasmonic resonances of the arrays are excited at the fundamental pump wavelength, thus boosting the intensity of the electromagnetic near-fields. Our experimental results, which are supported by numerical simulations of linear optical transmission and near-field enhancement spectra based on the Finite Difference Time Domain method, demonstrate a direct correlation between the onset of Fano-type coupling and the enhancement of second harmonic generation in arrays of Au nanoparticles. Our findings enable the engineering of the nonlinear optical response of Fano-type coupled nanoparticle arrays that are relevant to a number of device applications in nonlinear nano-optics and plasmonics, such as on-chip frequency generators, modulators, switchers, and sensors.

  4. Effect of hydrogenic impurity on the third-harmonic generation in a quantum well

    NASA Astrophysics Data System (ADS)

    Zhang, Zhongmin; Guo, Kangxian; Mou, Sen; Xiao, Bo; Liao, Lei

    2014-12-01

    The third-harmonic generation (THG) coefficients in a quantum well with hydrogenic impurity are theoretically investigated with the compact-density-matrix approach and iterative method. The wave functions and the energy levels can be obtained by using variational method and numerical method. Numerical results show that the THG coefficients are strongly affected by the hydrogenic impurity.

  5. Second-harmonic generation excited by a rotating Laguerre-Gaussian beam

    SciTech Connect

    Petrov, Dmitri

    2010-09-15

    Experimental data demonstrate that unlike linear optical processes, an optical Laguerre-Gaussian beam of frequency {omega}, with topological charge m, rotating with angular frequency {Omega}<<{omega}, may not be considered as a monochromatic beam with the shifted frequency {omega}+m{Omega} (Doppler angular shift) for the second-harmonic generation nonlinear process.

  6. Two-pass-internal second-harmonic generation using a prism coupler.

    NASA Technical Reports Server (NTRS)

    Gonzalez, D. G.; Nieh, S. T. K.; Steier, W. H.

    1973-01-01

    A dispersive quartz prism is used to couple the total second harmonic generated in both directions by an internal cavity frequency doubler. The study shows that the dispersion of air and mirror reflection phase shifts can be compensated for by a slight nonphase match condition in the doubler.

  7. Real-time observation of interfering crystal electrons in high-harmonic generation.

    PubMed

    Hohenleutner, M; Langer, F; Schubert, O; Knorr, M; Huttner, U; Koch, S W; Kira, M; Huber, R

    2015-07-30

    Acceleration and collision of particles has been a key strategy for exploring the texture of matter. Strong light waves can control and recollide electronic wavepackets, generating high-harmonic radiation that encodes the structure and dynamics of atoms and molecules and lays the foundations of attosecond science. The recent discovery of high-harmonic generation in bulk solids combines the idea of ultrafast acceleration with complex condensed matter systems, and provides hope for compact solid-state attosecond sources and electronics at optical frequencies. Yet the underlying quantum motion has not so far been observable in real time. Here we study high-harmonic generation in a bulk solid directly in the time domain, and reveal a new kind of strong-field excitation in the crystal. Unlike established atomic sources, our solid emits high-harmonic radiation as a sequence of subcycle bursts that coincide temporally with the field crests of one polarity of the driving terahertz waveform. We show that these features are characteristic of a non-perturbative quantum interference process that involves electrons from multiple valence bands. These results identify key mechanisms for future solid-state attosecond sources and next-generation light-wave electronics. The new quantum interference process justifies the hope for all-optical band-structure reconstruction and lays the foundation for possible quantum logic operations at optical clock rates. PMID:26223624

  8. Rydberg-Rydberg interaction in the second-harmonic generation from rubidium atoms

    SciTech Connect

    Melo, Natalia R. de; Vianna, Sandra S.

    2008-02-15

    We report on the observation of long range interaction in the second-harmonic generation from rubidium Rydberg atoms. The asymmetric spectral broadening of the resonant lines provides evidence of the van der Waals interaction between pairs of Rydberg atoms. This effect is investigated when the two-photon transition is resonant with nd levels for n{approx_equal}13.

  9. Homoclinic orbits and chaos in a second-harmonic generating optical cavity

    SciTech Connect

    Holm, D.; Kovacic, G., Timofeyev, I.

    1997-04-01

    We present two large families of Silnikov-type homoclinic orbits in a two mode-model that describes second-harmonic generation in a passive optical cavity. These families of homoclinic orbits give rise to chaotic dynamics in the model. 4 refs., 1 fig.

  10. Second harmonic generation of spectrally broadened femtosecond ytterbium laser radiation in a gas-filled capillary

    SciTech Connect

    Didenko, N V; Konyashchenko, Aleksandr V; Kostryukov, P V; Losev, Leonid L; Tenyakov, S Yu

    2011-09-30

    A 300-fs radiation pulse of an ytterbium laser with a wavelength of 1030 nm and energy of 150 {mu}J were converted to a 15-fs pulse with a wavelength of 515 nm by broadening the emission spectrum in a capillary filled with xenon and by generating the second harmonic in a KDP crystal. The energy efficiency of the conversion was 30 %.

  11. Second-harmonic generation of a new chalcone-type crystal

    NASA Astrophysics Data System (ADS)

    Zhang, G. J.; Kinoshita, T.; Sasaki, K.; Goto, Y.; Nakayama, M.

    1990-07-01

    A new type of chalcone crystal was prepared. Anisotropic indices with wavelength dispersion were measured by the Brewster angle method. The two largest second-harmonic generation (SHG) tensor components were determined by the wedge method and compared with d11 of 2-methyl-4-nitroaniline. Calculated collinear and noncollinear phase-matched SHG patterns reasonably fit the observed photographs.

  12. Optical generation of a circular harmonic filter for rotation and translation invariant optical pattern recognition

    NASA Technical Reports Server (NTRS)

    Cheng, Yeou-Yen

    1987-01-01

    A new method to generate a circular harmonic filter with both rotation and translation invariance is described, which is based on a phase-shifted double-exposure (PSDE) technique. An expression for the peak correlation intensity at the origin for the correlation plane as a function of target orientation for the PSDE filter is derived. Experimental results confirming the theoretical predictions are provided.

  13. First-principle description for the high-harmonic generation in a diamond by intense short laser pulse

    NASA Astrophysics Data System (ADS)

    Otobe, T.

    2012-05-01

    We present a first-principles description for the electron excitation and the high-harmonic generation (HHG) in a diamond by intense laser pulse irradiation and their laser parameter dependence. Above band gap harmonics are generated after the peak of the incident laser pulse and have duration much shorter than the laser pulse. The intensity of individual harmonic peaks increases as laser intensity increases nonlinearly, and we find the blue shift of the HHG spectrum when the optical breakdown occurs.

  14. Model of high-order harmonic generation from laser interaction with a plasma grating.

    PubMed

    Zhang, S J; Zhuo, H B; Zou, D B; Gan, L F; Zhou, H Y; Li, X Z; Yu, M Y; Yu, W

    2016-05-01

    Harmonic generation from linearly polarized high-intensity short-pulse laser normally impacting a solid plasma grating is investigated using analytical modeling and particle-in-cell simulation. It is found that when the radiation excited by the relativistic electron quiver motion in the laser fields suitably matches a harmonic of the grating periodicity, it will be significantly enhanced and peak with narrow angular spread in specific directions. The corresponding theory shows that the phenomenon can be attributed to an interference effect of the periodic grating on the excitation.

  15. Ultrashort pulse chirp measurement via transverse second-harmonic generation in strontium barium niobate crystal

    SciTech Connect

    Trull, J.; Wang, B.; Parra, A.; Vilaseca, R.; Cojocaru, C.; Sola, I.; Sheng, Y.

    2015-06-01

    Pulse compression in dispersive strontium barium niobate crystal with a random size and distribution of the anti-parallel orientated nonlinear domains is observed via transverse second harmonic generation. The dependence of the transverse width of the second harmonic trace along the propagation direction allows for the determination of the initial chirp and duration of pulses in the femtosecond regime. This technique permits a real-time analysis of the pulse evolution and facilitates fast in-situ correction of pulse chirp acquired in the propagation through an optical system.

  16. Model of high-order harmonic generation from laser interaction with a plasma grating

    NASA Astrophysics Data System (ADS)

    Zhang, S. J.; Zhuo, H. B.; Zou, D. B.; Gan, L. F.; Zhou, H. Y.; Li, X. Z.; Yu, M. Y.; Yu, W.

    2016-05-01

    Harmonic generation from linearly polarized high-intensity short-pulse laser normally impacting a solid plasma grating is investigated using analytical modeling and particle-in-cell simulation. It is found that when the radiation excited by the relativistic electron quiver motion in the laser fields suitably matches a harmonic of the grating periodicity, it will be significantly enhanced and peak with narrow angular spread in specific directions. The corresponding theory shows that the phenomenon can be attributed to an interference effect of the periodic grating on the excitation.

  17. Anomalous-dispersion phase-matched second-harmonic generation in a polymer waveguide

    SciTech Connect

    Kowalczyk, T.C.; Singer, K.D.; Cahill, P.A.

    1995-11-15

    We demonstrate phase-matched second-harmonic generation in a poled polymer waveguide, using anomalous-dispersion phase matching. Phase matching was achieved between lowest-order fundamental and harmonic modes, TM{sub 0}{sup {omega}} to TM{sub 0}{sup 2{omega}}, at a fundamental wavelength of 815 nm over a propagation length of 32 {mu}m. The maximum conversion efficiency was {eta}{sub exp}=39%/Wcm{sup 2}, in good agreement with theory. {copyright} {ital 1995} {ital Optical} {ital Society} {ital of} {ital America}.

  18. Model of high-order harmonic generation from laser interaction with a plasma grating.

    PubMed

    Zhang, S J; Zhuo, H B; Zou, D B; Gan, L F; Zhou, H Y; Li, X Z; Yu, M Y; Yu, W

    2016-05-01

    Harmonic generation from linearly polarized high-intensity short-pulse laser normally impacting a solid plasma grating is investigated using analytical modeling and particle-in-cell simulation. It is found that when the radiation excited by the relativistic electron quiver motion in the laser fields suitably matches a harmonic of the grating periodicity, it will be significantly enhanced and peak with narrow angular spread in specific directions. The corresponding theory shows that the phenomenon can be attributed to an interference effect of the periodic grating on the excitation. PMID:27300994

  19. Analysis of second-harmonic generation by primary ultrasonic guided wave propagation in a piezoelectric plate.

    PubMed

    Deng, Mingxi; Xiang, Yanxun

    2015-08-01

    The effect of second-harmonic generation (SHG) by primary ultrasonic guided wave propagation is analyzed, where the nonlinear elastic, piezoelectric, and dielectric properties of the piezoelectric plate material are considered simultaneously. The formal solution of the corresponding second-harmonic displacement field is presented. Theoretical and numerical investigations clearly show that the SHG effect of primary guided wave propagation is highly sensitive to the electrical boundary conditions of the piezoelectric plate. The results obtained may provide a means through which the SHG efficiency of ultrasonic guided wave propagation can effectively be regulated by changing the electrical boundary conditions of the piezoelectric plate.

  20. Interplay of mulitphoton and tunneling ionization in short-wavelength-driven high-order harmonic generation

    SciTech Connect

    Gkortsas, Vasileios-Marios; Bhardwaj, Siddharth; Lai, Chien-Jen; Hong, Kyung-Han; Falcao-Filho, Edilson L.; Kaertner, Franz X.

    2011-07-15

    High-order harmonic generation efficiency is theoretically modeled and compared with experiments using 400 and 800 nm driver pulses. It is shown that, for a short drive wavelength and a Keldysh parameter larger than 1, the Ammosov-Delone-Krainov (ADK) ionization model does not give a good agreement between theory and experiment. Since the ADK ionization model only accounts for tunnel ionization, it underestimates the yield of low-order harmonics from the wings of the driver pulse. In contrast, the Yudin-Ivanov ionization model [Phys. Rev. A 64, 013409 (2001)], which accounts for both tunnel and multiphoton ionization, gives much better agreement with the experimental results.

  1. Analysis of second-harmonic generation by primary ultrasonic guided wave propagation in a piezoelectric plate.

    PubMed

    Deng, Mingxi; Xiang, Yanxun

    2015-08-01

    The effect of second-harmonic generation (SHG) by primary ultrasonic guided wave propagation is analyzed, where the nonlinear elastic, piezoelectric, and dielectric properties of the piezoelectric plate material are considered simultaneously. The formal solution of the corresponding second-harmonic displacement field is presented. Theoretical and numerical investigations clearly show that the SHG effect of primary guided wave propagation is highly sensitive to the electrical boundary conditions of the piezoelectric plate. The results obtained may provide a means through which the SHG efficiency of ultrasonic guided wave propagation can effectively be regulated by changing the electrical boundary conditions of the piezoelectric plate. PMID:25911148

  2. Planar second-harmonic generation with noncollinear pumps in disordered media.

    PubMed

    Roppo, Vito; Dumay, David; Trull, Jose; Cojocaru, Crina; Saltiel, Solomon M; Staliunas, Kestutis; Vilaseca, Ramon; Neshev, Dragomir N; Krolikowski, Wieslaw; Kivshar, Yuri S

    2008-09-01

    We study experimentally the process of the second harmonic generation by two noncollinear beams in quadratic nonlinear crystals with a disordered structure of ferroelectric domains. We show that the second-harmonic radiation is emitted in the form of two cones as well as in a plane representing the cross-correlation of the two fundamental pulses. We demonstrate the implementation of this parametric process for characterisation of femtosecond pulses, enabling the estimation of pulse width, chirp, and front tilt. This is achieved through monitoring the evolution of the autocorrelation trace inside the nonlinear crystal.

  3. Whispering gallery microresonators for second harmonic light generation from a low number of small molecules.

    PubMed

    Dominguez-Juarez, J L; Kozyreff, G; Martorell, Jordi

    2011-01-01

    Unmarked sensitive detection of molecules is needed in environmental pollution monitoring, disease diagnosis, security screening systems and in many other situations in which a substance must be identified. When molecules are attached or adsorbed onto an interface, detecting their presence is possible using second harmonic light generation, because at interfaces the inversion symmetry is broken. However, such light generation usually requires either dense matter or a large number of molecules combined with high-power laser sources. Here we show that using high-Q spherical microresonators and low average power, between 50 and 100 small non-fluorescent molecules deposited on the outer surface of the microresonator can generate a detectable change in the second harmonic light. This generation requires phase matching in the whispering gallery modes, which we achieved using a new procedure to periodically pattern, with nanometric precision, a molecular surface monolayer. PMID:21448153

  4. Probe of Multielectron Dynamics in Xenon by Caustics in High-Order Harmonic Generation.

    PubMed

    Faccialà, D; Pabst, S; Bruner, B D; Ciriolo, A G; De Silvestri, S; Devetta, M; Negro, M; Soifer, H; Stagira, S; Dudovich, N; Vozzi, C

    2016-08-26

    We investigated the giant resonance in xenon by high-order harmonic generation spectroscopy driven by a two-color field. The addition of a nonperturbative second harmonic component parallel to the driving field breaks the symmetry between neighboring subcycles resulting in the appearance of spectral caustics at two distinct cutoff energies. By controlling the phase delay between the two color components it is possible to tailor the harmonic emission in order to amplify and isolate the spectral feature of interest. In this Letter we demonstrate how this control scheme can be used to investigate the role of electron correlations that give birth to the giant resonance in xenon. The collective excitations of the giant dipole resonance in xenon combined with the spectral manipulation associated with the two-color driving field allow us to see features that are normally not accessible and to obtain a good agreement between the experimental results and the theoretical predictions. PMID:27610855

  5. High-order harmonic generation yielding tunable extreme-ultraviolet radiation of high spectral purity.

    PubMed

    Brandi, F; Neshev, D; Ubachs, W

    2003-10-17

    Production of extreme-ultraviolet radiation by high-order harmonic generation is demonstrated to yield unprecedented spectral purity of lambda/Delta lambda=2.5 x 10(5) at wavelengths covering the entire range 40-100 nm. Tunability and sub-cm(-1) bandwidth of the harmonics are demonstrated in recordings of the He (1s4p) and Ar (3p(5)3d') resonance lines at 52.2 and 86.6 nm. Frequency shift of the harmonics due to chirp-induced phenomena are investigated and found to be small, resulting in a frequency accuracy of about 5 x 10(-7) in the domain of extreme-ultraviolet radiation.

  6. Enhancement of high harmonic generation by confining electron motion in plasmonic nanostrutures.

    PubMed

    Ciappina, M F; Aćimović, Srdjan S; Shaaran, T; Biegert, J; Quidant, R; Lewenstein, M

    2012-11-19

    We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse of long wavelength. We demonstrate that both the confinement of the electron motion and the inhomogeneous character of the laser electric field play an important role in the HHG process and lead to a significant increase of the harmonic cutoff. In particular, in bow-tie nanostructures with small gaps, electron trajectories with large excursion amplitudes experience significant confinement and their contribution is essentially suppressed. In order to understand and characterize this feature, we combine the numerical solution of the time-dependent Schrödinger equation (TDSE) with the electric fields obtained from 3D finite element simulations. We employ time-frequency analysis to extract more detailed information from the TDSE results and classical tools to explain the extended harmonic spectra. The spatial inhomogeneity of the laser electric field modifies substantially the electron trajectories and contributes also to cutoff increase.

  7. Two-Dimensional Frequency Resolved Optomolecular Gating of High-Order Harmonic Generation.

    PubMed

    Ferré, A; Soifer, H; Pedatzur, O; Bourassin-Bouchet, C; Bruner, B D; Canonge, R; Catoire, F; Descamps, D; Fabre, B; Mével, E; Petit, S; Dudovich, N; Mairesse, Y

    2016-02-01

    Probing electronic wave functions of polyatomic molecules is one of the major challenges in high-harmonic spectroscopy. The extremely nonlinear nature of the laser-molecule interaction couples the multiple degrees of freedom of the probed system. We combine two-dimensional control of the electron trajectories and vibrational control of the molecules to disentangle the two main steps in high-harmonic generation-ionization and recombination. We introduce a new measurement scheme, frequency-resolved optomolecular gating, which resolves the temporal amplitude and phase of the harmonic emission from excited molecules. Focusing on the study of vibrational motion in N_{2}O_{4}, we show that such advanced schemes provide a unique insight into the structural and dynamical properties of the underlying mechanism.

  8. Carrier-wave Rabi-flopping signatures in high-order harmonic generation for alkali atoms.

    PubMed

    Ciappina, M F; Pérez-Hernández, J A; Landsman, A S; Zimmermann, T; Lewenstein, M; Roso, L; Krausz, F

    2015-04-10

    We present a theoretical investigation of carrier-wave Rabi flopping in real atoms by employing numerical simulations of high-order harmonic generation (HHG) in alkali species. Given the short HHG cutoff, related to the low saturation intensity, we concentrate on the features of the third harmonic of sodium (Na) and potassium (K) atoms. For pulse areas of 2π and Na atoms, a characteristic unique peak appears, which, after analyzing the ground state population, we correlate with the conventional Rabi flopping. On the other hand, for larger pulse areas, carrier-wave Rabi flopping occurs, and is associated with a more complex structure in the third harmonic. These characteristics observed in K atoms indicate the breakdown of the area theorem, as was already demonstrated under similar circumstances in narrow band gap semiconductors. PMID:25910125

  9. Probe of Multielectron Dynamics in Xenon by Caustics in High-Order Harmonic Generation.

    PubMed

    Faccialà, D; Pabst, S; Bruner, B D; Ciriolo, A G; De Silvestri, S; Devetta, M; Negro, M; Soifer, H; Stagira, S; Dudovich, N; Vozzi, C

    2016-08-26

    We investigated the giant resonance in xenon by high-order harmonic generation spectroscopy driven by a two-color field. The addition of a nonperturbative second harmonic component parallel to the driving field breaks the symmetry between neighboring subcycles resulting in the appearance of spectral caustics at two distinct cutoff energies. By controlling the phase delay between the two color components it is possible to tailor the harmonic emission in order to amplify and isolate the spectral feature of interest. In this Letter we demonstrate how this control scheme can be used to investigate the role of electron correlations that give birth to the giant resonance in xenon. The collective excitations of the giant dipole resonance in xenon combined with the spectral manipulation associated with the two-color driving field allow us to see features that are normally not accessible and to obtain a good agreement between the experimental results and the theoretical predictions.

  10. Two-Dimensional Frequency Resolved Optomolecular Gating of High-Order Harmonic Generation.

    PubMed

    Ferré, A; Soifer, H; Pedatzur, O; Bourassin-Bouchet, C; Bruner, B D; Canonge, R; Catoire, F; Descamps, D; Fabre, B; Mével, E; Petit, S; Dudovich, N; Mairesse, Y

    2016-02-01

    Probing electronic wave functions of polyatomic molecules is one of the major challenges in high-harmonic spectroscopy. The extremely nonlinear nature of the laser-molecule interaction couples the multiple degrees of freedom of the probed system. We combine two-dimensional control of the electron trajectories and vibrational control of the molecules to disentangle the two main steps in high-harmonic generation-ionization and recombination. We introduce a new measurement scheme, frequency-resolved optomolecular gating, which resolves the temporal amplitude and phase of the harmonic emission from excited molecules. Focusing on the study of vibrational motion in N_{2}O_{4}, we show that such advanced schemes provide a unique insight into the structural and dynamical properties of the underlying mechanism. PMID:26894708

  11. High-order harmonic generation in polyatomic molecules induced by a bicircular laser field

    NASA Astrophysics Data System (ADS)

    Odžak, S.; Hasović, E.; Milošević, D. B.

    2016-09-01

    High-order harmonic generation by a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency r ω and s ω (r and s are integers), is investigated for a polyatomic molecule. This field possesses dynamical symmetry, which can be adjusted to the symmetry of the molecular Hamiltonian and used to investigate the molecular symmetry. For polyatomic molecules having the Cr +s symmetry, only the harmonics n =q (r +s )±r ,q =1 ,2 ,..., are emitted having the ellipticity ɛn=±1 . We illustrate this using the example of the planar molecules BH3 and BF3, which obey the C3 symmetry. We show that for the BF3 molecule, similarly to atoms with a p ground state, there is a strong asymmetry in the emission of high harmonics with opposite helicities. This asymmetry depends on the molecular orientation.

  12. Carrier-wave Rabi-flopping signatures in high-order harmonic generation for alkali atoms.

    PubMed

    Ciappina, M F; Pérez-Hernández, J A; Landsman, A S; Zimmermann, T; Lewenstein, M; Roso, L; Krausz, F

    2015-04-10

    We present a theoretical investigation of carrier-wave Rabi flopping in real atoms by employing numerical simulations of high-order harmonic generation (HHG) in alkali species. Given the short HHG cutoff, related to the low saturation intensity, we concentrate on the features of the third harmonic of sodium (Na) and potassium (K) atoms. For pulse areas of 2π and Na atoms, a characteristic unique peak appears, which, after analyzing the ground state population, we correlate with the conventional Rabi flopping. On the other hand, for larger pulse areas, carrier-wave Rabi flopping occurs, and is associated with a more complex structure in the third harmonic. These characteristics observed in K atoms indicate the breakdown of the area theorem, as was already demonstrated under similar circumstances in narrow band gap semiconductors.

  13. Probe of Multielectron Dynamics in Xenon by Caustics in High-Order Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Faccialà, D.; Pabst, S.; Bruner, B. D.; Ciriolo, A. G.; De Silvestri, S.; Devetta, M.; Negro, M.; Soifer, H.; Stagira, S.; Dudovich, N.; Vozzi, C.

    2016-08-01

    We investigated the giant resonance in xenon by high-order harmonic generation spectroscopy driven by a two-color field. The addition of a nonperturbative second harmonic component parallel to the driving field breaks the symmetry between neighboring subcycles resulting in the appearance of spectral caustics at two distinct cutoff energies. By controlling the phase delay between the two color components it is possible to tailor the harmonic emission in order to amplify and isolate the spectral feature of interest. In this Letter we demonstrate how this control scheme can be used to investigate the role of electron correlations that give birth to the giant resonance in xenon. The collective excitations of the giant dipole resonance in xenon combined with the spectral manipulation associated with the two-color driving field allow us to see features that are normally not accessible and to obtain a good agreement between the experimental results and the theoretical predictions.

  14. Harmonic generation in the discrete spectral region of xenon using broadband femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Kutzner, J.; Tsilimis, G.; Zacharias, H.

    2005-02-01

    The conversion of 34-fs Ti:sapphire laser pulses into the wavelength region 105 210 nm has been studied in xenon for laser intensities up to 5×1013 W/cm2. A strongly structured, pressure-dependent emission spectrum is observed. Radiation is detected in regions expected for the 5th and 7th harmonics but also in regions in between. In the resonance region (λ<147 nm), self-phase-modulation processes in the conversion medium together with phase-matched, efficient harmonic generation in negative-dispersive spectral regions explain the observations. Broadband emission is detected in the resonance-free, positive-dispersive spectral region 155 210 nm. Emission from the xenon dimer is superimposed on a ‘direct’ 5th-harmonic signal.

  15. Analytic model of bunched beams for harmonic generation in thelow-gain free electron laser regime

    SciTech Connect

    Penn, G.; Reinsch, M.; Wurtele, J.S.

    2006-02-20

    One scheme for harmonic generation employs free electron lasers (FELs) with two undulators: the first uses a seed laser to modulate the energy of the electron beam; following a dispersive element which acts to bunch the beam, the second undulator radiates at a higher harmonic. These processes are currently evaluated using extensive calculations or simulation codes which can be slow to evaluate and difficult to set up. We describe a simple algorithm to predict the output of a harmonic generation beamline in the low-gain FEL regime, based on trial functions for the output radiation. Full three-dimensional effects are included. This method has been implemented as a Mathematica package, named CAMPANILE, which runs rapidly and can be generalized to include effects such as asymmetric beams and misalignments. This method is compared with simulation results using the FEL code GENESIS, both for single stages of harmonic generation and for the LUX project, a design concept for an ultrafast X-ray facility, where multiple stages upshift the input laser frequency by factors of up to 200.

  16. X-ray FEL based on harmonics generation and electron beam outcoupling

    SciTech Connect

    Litvinenko, V.N.; Burnham, B.

    1995-12-31

    Electron beam outcoupling was suggested by N. A. Vinokurov as a method of optics independent outcoupling for high power FELs. The bunching of the electron beam is provided in a master oscillator. The prebunched electron beam then radiates coherently into an additional wiggler called the radiator. The electron beam is turned by an achromatic bend into this wiggler and its radiation propagates with a small angle with respect to the OK-4 optical axis. Thus, the radiation will pass around the mirror of the master oscillator optical cavity and can then be utilized. This scheme is perfectly suited for harmonic generation if the radiator wiggler is tuned on one of the master oscillator wavelength harmonics. This system is reminiscent of a klystron operating on a harmonic of the reference frequency. In this paper we present the theory of this device, its spectral and spatial characteristics of radiation, the optimization of the master oscillator, the achromatic bend and bunching for harmonic generation, and influence of beam parameters (energy spread, emittance, etc.) on generated power. Examples of possible storage ring and linac driven systems are discussed.

  17. Two-dimensional phase transformation probed by second harmonic generation: Oscillatory transformation of the K/Al(111) system

    SciTech Connect

    Ying, Z.C.; Plummer, E.W. |

    1995-12-31

    The technique of optical second harmonic generation is used to study phase transformations at two-dimensional surfaces and interfaces. Examples are given to illustrate that changes in surface symmetry, adsorption configuration, and electronic structure can be detected by this nonlinear optical technique. An oscillatory phase transformation of potassium adsorbed atoms on Al(111) probed by second harmonic generation is analyzed in detail.

  18. Generation Of 369.4-Nanometers Second Harmonic From A Diode Laser

    NASA Technical Reports Server (NTRS)

    Williams, Angelyn P.; Maleki, Lutfollah

    1995-01-01

    Experimental laser system features polarization feedback scheme maintaining frequency lock. Generates light at wavelength of 369.4 nanometers by second-harmonic generation from 738.8-nanometers laser diode. System prototype of source of 369.4-nanometers radiation used to optically pump 2S1/2 ' 2P1/2 transition in 171Yb+ ions in lightweight, low-power trapped-ion frequency-standard apparatus.

  19. Extreme-ultraviolet polarimeter utilizing laser-generated high-order harmonics.

    PubMed

    Brimhall, Nicole; Turner, Matthew; Herrick, Nicholas; Allred, David D; Turley, R Steven; Ware, Michael; Peatross, Justin

    2008-10-01

    We describe an extreme-ultraviolet (EUV) polarimeter that employs laser-generated high-order harmonics as the light source. The polarimeter is designed to characterize materials and thin films for use with EUV light. Laser high harmonics are highly directional with easily rotatable linear polarization, not typically available with other EUV sources. The harmonics have good wavelength coverage, potentially spanning the entire EUV from a few to a hundred nanometers. Our instrument is configured to measure reflectances from 14 to 30 nm and has approximately 180 spectral resolution (lambda/Delta lambda). The reflection from a sample surface can be measured over a continuous range of incident angles (5 degrees-75 degrees). A secondary 14 cm gas cell attenuates the harmonics in a controlled way to keep signals within the linear dynamic range of the detector, comprised of a microchannel plate coupled to a phosphorous screen and charge coupled device camera. The harmonics are produced using approximately 10 mJ, approximately 35 fs, and approximately 800 nm laser pulses with a repetition rate of 10 Hz. Per-shot energy monitoring of the laser discriminates against fluctuations. The polarimeter reflectance data agree well with data obtained at the Advanced Light Source Synchrotron (Beamline 6.3.2).

  20. Construction of an extreme ultraviolet polarimeter based on high-order harmonic generation

    NASA Astrophysics Data System (ADS)

    Brimhall, N.; Painter, J. C.; Turner, M.; Voronov, S. V.; Turley, R. S.; Ware, M.; Peatross, J.

    2006-08-01

    We report on the development of a polarimeter for characterizing reflective surfaces throughout the extreme ultraviolet (EUV). The instrument relies on laser high-order harmonics generated in helium, neon, or argon gas. The 800 nm laser generates a discrete comb of odd harmonics up to order 100 (wavelengths from 8-62 nm). The flux of EUV light is a couple orders of magnitude less than a synchrotron source but 30,000 times greater than a plasma source currently in operation at BYU. The polarimeter determines the reflectance from surfaces as a function of incident angle, linear light polarization orientation, and wavelength. The instrument uses a wave plate in the laser beam to control the orientation of the harmonic polarization (linear, same as laser). After reflecting from the sample, the harmonic beams are dispersed by a grating and focused onto a micro-channel plate coupled to a phosphor screen. We have demonstrated the feasibility of this project with a simple prototype instrument, which measured the reflectance of samples from 30 nm to 62 nm. The prototype demonstrated that sensitivity is sufficient for measuring reflectances as low as 0.5% for both s- and p-polarized light. The full instrument employs extensive scanning mobility as opposed to the fixed angle and fixed wavelength range of our earlier prototype. An advantage of employing harmonics as a source for EUV polarimetry is that a wide range of wavelengths can be measured simultaneously. This project represents an authentic 'work-horse' application for high-order harmonics, as opposed to merely demonstrating proof of concept.

  1. Low- and high-order harmonic generation in the extended plasmas produced by laser ablation of zinc and manganese targets

    SciTech Connect

    Ganeev, R. A.; Baba, M.; Suzuki, M.; Yoneya, S.; Kuroda, H.

    2014-12-28

    The systematic studies of the harmonic generation of ultrashort laser pulses in the 5-mm-long Zn and Mn plasmas (i.e., application of nanosecond, picosecond, and femtosecond pulses for ablation, comparison of harmonic generation from atomic, ionic, and cluster-contained species of plasma, variation of plasma length, two-color pump of plasmas, etc.) are presented. The conversion efficiency of the 11th–19th harmonics generated in the Zn plasma was ∼5 × 10{sup −5}. The role of the ionic resonances of Zn near the 9th and 10th harmonics on the enhancement of harmonics is discussed. The enhancement of harmonics was also analyzed using the two-color pump of extended plasmas, which showed similar intensities of the odd and even harmonics along the whole range of generation. The harmonics up to the 107th order were demonstrated in the case of manganese plasma. The comparison of harmonic generation in the 5-mm-long and commonly used short (≤0.5 mm) plasma plumes showed the advanced properties of extended media.

  2. Second-harmonic generation in shear wave beams with different polarizations

    SciTech Connect

    Spratt, Kyle S. Ilinskii, Yurii A.; Zabolotskaya, Evgenia A.; Hamilton, Mark F.

    2015-10-28

    A coupled pair of nonlinear parabolic equations was derived by Zabolotskaya [1] that model the transverse components of the particle motion in a collimated shear wave beam propagating in an isotropic elastic solid. Like the KZK equation, the parabolic equation for shear wave beams accounts consistently for the leading order effects of diffraction, viscosity and nonlinearity. The nonlinearity includes a cubic nonlinear term that is equivalent to that present in plane shear waves, as well as a quadratic nonlinear term that is unique to diffracting beams. The work by Wochner et al. [2] considered shear wave beams with translational polarizations (linear, circular and elliptical), wherein second-order nonlinear effects vanish and the leading order nonlinear effect is third-harmonic generation by the cubic nonlinearity. The purpose of the current work is to investigate the quadratic nonlinear term present in the parabolic equation for shear wave beams by considering second-harmonic generation in Gaussian beams as a second-order nonlinear effect using standard perturbation theory. In order for second-order nonlinear effects to be present, a broader class of source polarizations must be considered that includes not only the familiar translational polarizations, but also polarizations accounting for stretching, shearing and rotation of the source plane. It is found that the polarization of the second harmonic generated by the quadratic nonlinearity is not necessarily the same as the polarization of the source-frequency beam, and we are able to derive a general analytic solution for second-harmonic generation from a Gaussian source condition that gives explicitly the relationship between the polarization of the source-frequency beam and the polarization of the second harmonic.

  3. Experimental observation of fundamental and harmonic self pulse generation of single high-order Stokes in Brillouin Erbium fiber laser

    NASA Astrophysics Data System (ADS)

    Wang, Xiaorui; Yang, Yanfu; Liu, Meng; Yao, Yong

    2016-07-01

    Fundamental and harmonic self-pulse generation was experimentally observed on both first order and higher order Stokes components. The generated pulses with the same order harmonic repetition rate are obtained on multiple Stokes components simultaneously. The pulse generation on first order Stokes component can be attributed to periodic pump depletion in Brillouin gain medium. The pulse generation of high order Stokes component can be considered as pulse oscillation pumped by the former order Stokes. With high Erbium pump power, by setting the proper attenuation between Brillouin medium and Faraday rotation mirror, the harmonic pulse generations up to fifth order have been achieved.

  4. Progress toward high-gain laser fusion

    SciTech Connect

    Storm, E.

    1988-09-28

    A 1985-1986 Review of the US inertial confinement fusion program by the National Academy of Sciences concluded that five more years might be required to obtain enough data to determine the future course of the program. Since then, data from the Nova laser and from the Halite/Centurion program have resolved most of the outstanding problems identified by the NAS review. In particular, we now believe that we can produce a sufficiently uniform target; that we can keep the energy content in hot electrons and high-energy photons low enough (/approximately/1--10% of drive energy, depending on target design) and achieve enough pulse-shaping accuracy (/approximately/10%, with a dynamic range of 100:1) to keep the fuel on a near-Fermi-degenerate adiabat; that we can produce an /approximately/100-Mbar pressure pulse of sufficient uniformity (/approximately/1%), and can we control hydrodynamic instabilities so that the mix of the pusher into the hot spot is low enough to permit marginal ignition. These results are sufficiently encouraging that the US Department of Energy is planning to complete a 10-MJ laboratory microfusion facility to demonstrate high-gain ICF in the laboratory within a decade. 22 refs., 1 fig.

  5. Bright high-order harmonic generation with controllable polarization from a relativistic plasma mirror.

    PubMed

    Chen, Zi-Yu; Pukhov, Alexander

    2016-01-01

    Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still limited to only a few free-electron laser facilities and, very recently, to high-order harmonic generation from noble gases. Here we propose and numerically demonstrate a laser-plasma scheme to generate bright XUV pulses with fully controlled polarization. In this scheme, an elliptically polarized laser pulse is obliquely incident on a plasma surface, and the reflected radiation contains pulse trains and isolated circularly or highly elliptically polarized attosecond XUV pulses. The harmonic polarization state is fully controlled by the laser-plasma parameters. The mechanism can be explained within the relativistically oscillating mirror model. This scheme opens a practical and promising route to generate bright attosecond XUV pulses with desirable ellipticities in a straightforward and efficient way for a number of applications. PMID:27531047

  6. Bright high-order harmonic generation with controllable polarization from a relativistic plasma mirror

    PubMed Central

    Chen, Zi-Yu; Pukhov, Alexander

    2016-01-01

    Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still limited to only a few free-electron laser facilities and, very recently, to high-order harmonic generation from noble gases. Here we propose and numerically demonstrate a laser–plasma scheme to generate bright XUV pulses with fully controlled polarization. In this scheme, an elliptically polarized laser pulse is obliquely incident on a plasma surface, and the reflected radiation contains pulse trains and isolated circularly or highly elliptically polarized attosecond XUV pulses. The harmonic polarization state is fully controlled by the laser–plasma parameters. The mechanism can be explained within the relativistically oscillating mirror model. This scheme opens a practical and promising route to generate bright attosecond XUV pulses with desirable ellipticities in a straightforward and efficient way for a number of applications. PMID:27531047

  7. Role of long quantum orbits in high-order harmonic generation

    SciTech Connect

    Milosevic, D.B.; Becker, W.

    2002-12-01

    Single-atom high-order harmonic generation is considered in the strong-field approximation, as formulated in the Lewenstein model, and analyzed in terms of quantum orbits. Orbits are classified according to the solutions of the saddle-point equations. The results of a numerical integration are compared with the saddle-point approximation and the uniform approximation. Approximate analytical solutions for long orbits are presented. The formalism developed is used to analyze the enhancement of high-order harmonic generation near channel closings. The enhancements exactly at the channel closings are extremely narrow and built up by the constructive interference of a very large number of quantum orbits. Additional broader enhancements occur slightly below channel closings. They are generated by the interplay of a medium number of orbits.

  8. Dot patterns from second-harmonic and sum-frequency generation in polycrystalline ZnSe

    NASA Astrophysics Data System (ADS)

    Chinh, Tran Duc; Seibt, Wolfgang; Siegbahn, Kai

    2001-09-01

    During a comparative study of second-harmonic generation (SHG) and sum-frequency generation (SFG) in single-crystal and polycrystalline ZnSe, the polycrystalline material showed a dot pattern in the SHG as well as in the SFG output. No such pattern was found in the output from the single-crystal ZnSe sample. The second-harmonic and also the sum-frequency dot pattern, resembling a diffraction pattern, could be observed over a wide tuning range of the fundamental beam, between 1.1 and 1.6 μm, generated by a femtosecond optical parametric amplifier. The size of the observed pattern is dependent on wavelength and the dots show a characteristic polarization.

  9. High energy diode pumped 5th harmonic generation of Nd: YAG laser

    NASA Astrophysics Data System (ADS)

    Yu, Yang; Cheng, Chee Yuen; Chia, Yong Poo; Wong, Wee Hoong; Yong, Saw Soon; Qu, Weijuan; Peng, Xiaoyuan

    2013-03-01

    This paper reports a high power diode pump 5th harmonic generation of Nd: YAG laser system, which could generate up to 300 mW TEM00 mode output with 100 Hz repetition rate at 213 nm. A diode pump module was specially designed for a high efficiency and good beam quality at the fundamental wavelength 1064 nm. An amplifier was set up out of the cavity to boost up the energy level of fundamental wavelength. In order to get high efficiency of the 5th harmonic generation, the cavity of the fundamental wavelength is EOM Q-switched which could generate very high peak power of the fundamental wavelength laser for extra cavity harmonic generations. Finally, 14% conversion efficiency from IR to UV was achieved, which is the highest efficiency in the market to the best of our knowledge right now. 213 nm is a very good substitute wavelength of 193 nm for different UV applications, the system of which is more compact, higher energy, less maintenance and better beam quality than the system of 193 nm.

  10. Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation.

    PubMed

    Celebrano, Michele; Wu, Xiaofei; Baselli, Milena; Großmann, Swen; Biagioni, Paolo; Locatelli, Andrea; De Angelis, Costantino; Cerullo, Giulio; Osellame, Roberto; Hecht, Bert; Duò, Lamberto; Ciccacci, Franco; Finazzi, Marco

    2015-05-01

    Boosting nonlinear frequency conversion in extremely confined volumes remains a challenge in nano-optics research, but can enable applications in nanomedicine, photocatalysis and background-free biosensing. To obtain brighter nonlinear nanoscale sources, approaches that enhance the electromagnetic field intensity and counter the lack of phase matching in nanoplasmonic systems are often employed. However, the high degree of symmetry in the crystalline structure of plasmonic materials (metals in particular) and in nanoantenna designs strongly quenches second harmonic generation. Here, we describe doubly-resonant single-crystalline gold nanostructures with no axial symmetry displaying spatial mode overlap at both the excitation and second harmonic wavelengths. The combination of these features allows the attainment of a nonlinear coefficient for second harmonic generation of ∼5 × 10(-10) W(-1), enabling a second harmonic photon yield higher than 3 × 10(6) photons per second. Theoretical estimations point toward the use of our nonlinear plasmonic nanoantennas as efficient platforms for label-free molecular sensing. PMID:25895003

  11. Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation

    NASA Astrophysics Data System (ADS)

    Celebrano, Michele; Wu, Xiaofei; Baselli, Milena; Großmann, Swen; Biagioni, Paolo; Locatelli, Andrea; de Angelis, Costantino; Cerullo, Giulio; Osellame, Roberto; Hecht, Bert; Duò, Lamberto; Ciccacci, Franco; Finazzi, Marco

    2015-05-01

    Boosting nonlinear frequency conversion in extremely confined volumes remains a challenge in nano-optics research, but can enable applications in nanomedicine, photocatalysis and background-free biosensing. To obtain brighter nonlinear nanoscale sources, approaches that enhance the electromagnetic field intensity and counter the lack of phase matching in nanoplasmonic systems are often employed. However, the high degree of symmetry in the crystalline structure of plasmonic materials (metals in particular) and in nanoantenna designs strongly quenches second harmonic generation. Here, we describe doubly-resonant single-crystalline gold nanostructures with no axial symmetry displaying spatial mode overlap at both the excitation and second harmonic wavelengths. The combination of these features allows the attainment of a nonlinear coefficient for second harmonic generation of ˜5 × 10-10 W-1, enabling a second harmonic photon yield higher than 3 × 106 photons per second. Theoretical estimations point toward the use of our nonlinear plasmonic nanoantennas as efficient platforms for label-free molecular sensing.

  12. Harmonization of initial estimates of shale gas life cycle greenhouse gas emissions for electric power generation.

    PubMed

    Heath, Garvin A; O'Donoughue, Patrick; Arent, Douglas J; Bazilian, Morgan

    2014-08-01

    Recent technological advances in the recovery of unconventional natural gas, particularly shale gas, have served to dramatically increase domestic production and reserve estimates for the United States and internationally. This trend has led to lowered prices and increased scrutiny on production practices. Questions have been raised as to how greenhouse gas (GHG) emissions from the life cycle of shale gas production and use compares with that of conventionally produced natural gas or other fuel sources such as coal. Recent literature has come to different conclusions on this point, largely due to differing assumptions, comparison baselines, and system boundaries. Through a meta-analytical procedure we call harmonization, we develop robust, analytically consistent, and updated comparisons of estimates of life cycle GHG emissions for electricity produced from shale gas, conventionally produced natural gas, and coal. On a per-unit electrical output basis, harmonization reveals that median estimates of GHG emissions from shale gas-generated electricity are similar to those for conventional natural gas, with both approximately half that of the central tendency of coal. Sensitivity analysis on the harmonized estimates indicates that assumptions regarding liquids unloading and estimated ultimate recovery (EUR) of wells have the greatest influence on life cycle GHG emissions, whereby shale gas life cycle GHG emissions could approach the range of best-performing coal-fired generation under certain scenarios. Despite clarification of published estimates through harmonization, these initial assessments should be confirmed through methane emissions measurements at components and in the atmosphere and through better characterization of EUR and practices.

  13. Rotating-frame perspective on high-order-harmonic generation of circularly polarized light

    NASA Astrophysics Data System (ADS)

    Reich, Daniel M.; Madsen, Lars Bojer

    2016-04-01

    We employ a rotating frame of reference to elucidate high-order-harmonic generation of circularly polarized light by bicircular driving fields. In particular, we show how the experimentally observed circular components of the high-order-harmonic spectrum can be directly related to the corresponding quantities in the rotating frame. Supported by numerical simulations of the time-dependent Schrödinger equation, we deduce an optimal strategy for maximizing the cutoff in the high-order-harmonic plateau while keeping the two circular components of the emitted light spectrally distinct. Moreover, we show how the rotating-frame picture can be more generally employed for elliptical drivers. Finally, we point out how circular and elliptical driving fields show a near-duality to static electric and magnetic fields in a rotating-frame description. This demonstrates how high-order-harmonic generation of circularly polarized light under static electromagnetic fields can be emulated in practice even at static field strengths beyond current experimental capabilities.

  14. Theoretical exploration of harmonic emission and attosecond pulse generation from H2+ in the presence of terahertz pulse

    NASA Astrophysics Data System (ADS)

    Liu, Hang; Feng, Liqiang

    2016-06-01

    Harmonic generation spectra from H2+ molecule ion driven by the chirped pulse combined with a terahertz (THz) pulse have been theoretically investigated by numerically solving the non-Born-Oppenheimer time-dependent Schrödinger equation (NBO-TDSE). The results show that with the introduction of the chirp, the harmonic cutoff is extended, resulting in a smooth supercontinuum. Further, when the initial vibrational state is prepared as v = 3, and by properly adding a THz controlling pulse, the harmonic yield is enhanced by almost six orders of magnitude compared with the single chirped pulse case. Quantum analyses are shown to explain the harmonic extension and enhancement. Furthermore, through the investigation of the isotopic effect, we find that more intense harmonics are generated in the lighter nucleus. Finally, by properly superposing the harmonics, a series of intense 35 as XUV pulses can be obtained, which are almost six orders of magnitude improvement in comparison with the single chirped pulse case.

  15. Noninvasive corneal stromal collagen imaging using two-photon-generated second-harmonic signals

    PubMed Central

    Morishige, Naoyuki; Petroll, W. Matthew; Nishida, Teruo; Kenney, M. Cristina; Jester, James V.

    2007-01-01

    PURPOSE To investigate the feasibility of using femtosecond-pulse lasers to produce second-harmonic generated (SHG) signals to noninvasively assess corneal stromal collagen organization. SETTING The Eye Institute, University of California, Irvine, California, USA. METHODS Mouse, rabbit, and human corneas were examined by two-photon confocal microscopy using a variable-wavelength femtosecond lasers to produce SHG signals. Two types were detected: forward scattered and backward scattered. Wavelength dependence of the SHG signal was confirmed by spectral separation using the 510 Meta (Zeiss). To verify the spatial relation between SHG signals and corneal cells, staining of cytoskeletons and nuclei was performed. RESULTS Second-harmonic-generated signal intensity was strongest with an excitation wavelength of 800 nm for all 3 species. Second-harmonic-generated forward signals showed a distinct fibrillar pattern organized into bands suggesting lamellae, while backscattered SHG signals appeared more diffuse and indistinct. Reconstruction of SHG signals showed two patterns of lamellar organization: highly interwoven in the anterior stroma and orthogonally arranged in the posterior stroma. Unique to the human cornea was the presence of transverse, sutural lamellae that inserted into Bowman’s layer, suggesting an anchoring function. CONCLUSIONS Using two-photon confocal microscopy to generate SHG signals from the corneal collagen provides a powerful new approach to noninvasively study corneal structure. Human corneas had a unique organizational pattern with sutural lamellae to provide important biomechanical support that was not present in mouse or rabbit corneas. PMID:17081858

  16. Investigation of the avalanche photodiodes for the CMS electromagnetic calorimeter operated at high gain

    NASA Astrophysics Data System (ADS)

    Deiters, K.; Diemoz, M.; Godinovic, N.; Ingram, Q.; Longo, E.; Montecchi, M.; Musienko, Y.; Nicol, S.; Patel, B.; Renker, D.; Reucroft, S.; Rusack, R.; Sakhelashvili, T.; Singovski, A.; Soric, I.; Swain, J.; Vikas, P.

    2001-04-01

    Avalanche Photodiodes (APD) with improved characteristics were developed by Hamamatsu Photonics for the Electromagnetic Calorimeter of the CMS experiment. This report presents measurements of the latest generation of APDs, which are capable to operate at high gains (˜2000).

  17. Phase-matched second-harmonic generation in poled polymers by the use of birefringence

    NASA Astrophysics Data System (ADS)

    Tao, X. T.; Watanabe, T.; Zou, D. C.; Ukuda, H.; Miyata, S.

    1995-09-01

    Green light has been observed for the first time to the authors' knowledge by bulk phase-matched second-harmonic generation from a stretched main chain polyurea. The polyurea was synthesized from 4,4'-diphenylmethane diisocyanate and 4,4'-methylene bis(cyclohexylamine). The spin-coated film has an initial positive birefringence. Drawing further increased the birefringence, and the film can be used for phase matching just as in biaxial single crystals. The drawn and poled polymer films belong to the 2mm point group. Three independent nonlinear-optic coefficients were determined. The type I phase-matching characteristics were calculated and confirmed by experiments. We demonstrate that a highly effective second-harmonic-generation device with a long optical path length can be obtained by use of bulk phase-matchable poled polymer.

  18. Higher harmonic generation in nonlinear waveguides of arbitrary cross-section.

    PubMed

    Srivastava, Ankit; Bartoli, Ivan; Salamone, Salvatore; Lanza di Scalea, Francesco

    2010-05-01

    This article concerns the generation and properties of double harmonics in nonlinear isotropic waveguides of complex cross-section. Analytical solutions of nonlinear Rayleigh-Lamb waves and rod waves have been known for some time. These solutions explain the phenomenon of cumulative double harmonic generation of guided waves. These solutions, however, are only applicable to simple geometries. This paper combines the general approach of the analytical solutions with semi-analytical finite element models to generalize the method to more complex geometries, specifically waveguides with arbitrary cross-sections. Supporting comparisons with analytical solutions are presented for simple cases. This is followed by the study of the case of a rail track. One reason for studying nonlinear guided waves in rails is the potential measurement of thermal stresses in welded rail.

  19. Generation of higher harmonics in longitudinal vibration of beams with breathing cracks

    NASA Astrophysics Data System (ADS)

    Broda, D.; Pieczonka, L.; Hiwarkar, V.; Staszewski, W. J.; Silberschmidt, V. V.

    2016-10-01

    Classical nonlinear vibration methods used for structural damage detection are often based on higher- and sub-harmonic generation. However, nonlinearities arising from sources other than damage - e.g. boundary conditions or a measurement chain - are a primary concern in these methods. This paper focuses on localisation of damage-related nonlinearities based on higher harmonic generation. Numerical and experimental investigations in longitudinal vibration of beams with breathing cracks are presented. Numerical modelling is performed using a two-dimensional finite element approach. Different crack depths, locations and boundary conditions are investigated. The results demonstrate that nonlinearities in cracked beams are particularly strong in the vicinity of damage, allowing not only for damage localisation but also for separation of crack induced nonlinearity from other sources of nonlinearities.

  20. Active control of highly efficient third-harmonic generation in ultrathin nonlinear metasurfaces

    NASA Astrophysics Data System (ADS)

    Gong, Zibo; Li, Chong; Hu, Xiaoyong; Yang, Hong; Gong, Qihuang

    2016-10-01

    Active electric control of highly efficient third harmonic generation was realized in an ultrathin nonlinear metasurface by using a nanocomposite consisting of gold nanoparticles dispersed in polycrystalline strontium titanate as the electro-optic material. Owing to the nonlinearity enhancement associated with the slow light effect, quantum confinement effect, and field-reinforcement, a high conversion efficiency of 3 × 10-5 was obtained, which is two orders of magnitude larger than previously reported efficiencies at comparable pump intensities. A modulation of 12% in the intensity of the third harmonic generation and a 30-nm shift in the transparency window center were achieved by varying the applied voltage from -30 V to zero. Our results pave the way toward the realization of multi-functional integrated photonic devices and chips based on metasurfaces.

  1. Multiple layer optical memory system using second-harmonic-generation readout

    DOEpatents

    Boyd, Gary T.; Shen, Yuen-Ron

    1989-01-01

    A novel optical read and write information storage system is described which comprises a radiation source such as a laser for writing and illumination, the radiation source being capable of radiating a preselected first frequency; a storage medium including at least one layer of material for receiving radiation from the radiation source and capable of being surface modified in response to said radiation source when operated in a writing mode and capable of generating a pattern of radiation of the second harmonic of the preselected frequency when illuminated by the radiation source at the preselected frequency corresponding to the surface modifications on the storage medium; and a detector to receive the pattern of second harmonic frequency generated.

  2. Efficient Co-Generation of Seventh-Harmonic Radiation in Cyclotron Autoresonance Acceleration

    SciTech Connect

    Wang, C.; Hirshfield, J.L.; Ganguly, A.K. |

    1996-10-01

    It is shown that the lowest TE{sub {ital s},{ital l}} mode in a cylindrical waveguide at frequency {ital s}{omega}, with group velocity nearly identical to group velocity for the TE{sub 11} mode at frequency {omega}, is that with {ital s}=7, {ital l}=2. This allows coherent radiation to be generated at the seventh harmonic during electron autoresonance acceleration. Conditions are found where such co-generation of 7th harmonic power at 20GHz is possible with overall efficiency greater than 80{percent}. This mechanism could make possible high efficiency cm-wavelength high power rf sources suitable for driving a future multi-TeV electron-position collider. {copyright} {ital 1996 The American Physical Society.}

  3. Electron path control of high-order harmonic generation by a spatially inhomogeneous field

    NASA Astrophysics Data System (ADS)

    Mohebbi, Masoud; Nazarpoor Malaei, Sakineh

    2016-04-01

    We theoretically investigate the control of high-order harmonics cut-off and as-pulse generation by a chirped laser field using a metallic bow tie-shaped nanostructure. The numerical results show that the trajectories of the electron wave packet are strongly modified, the short quantum path is enhanced, the long quantum path is suppressed and the low modulated spectrum of the harmonics can be remarkably extended. Our calculated results also show that, by confining electron motion, a broadband supercontinuum with the width of 1670 eV can be produced which directly generates an isolated 34 as-pulse without phase compensation. To explore the underlying mechanism responsible for the cut-off extension and the quantum path selection, we perform time-frequency analysis and a classical simulation based on the three-step model.

  4. Microwave frequency tuning and harmonic generation in ferroelectric thin film transmission lines

    NASA Astrophysics Data System (ADS)

    Booth, James C.; Ono, R. H.; Takeuchi, Ichiro; Chang, Kao-Shuo

    2002-07-01

    We evaluate dielectric tuning on nanosecond time scales in ferroelectric Ba0.3Sr0.7TiO3 thin films by measuring nonlinear harmonic generation at a fundamental frequency of 3 GHz. We compare the form of the distributed nonlinear capacitance per unit length C(Vrf) extracted from a simple model of harmonic generation in coplanar waveguide transmission line structures with the nonlinear capacitance C(Vdc) measured using a dc bias voltage, and obtain excellent agreement for temperatures in the range 235-295 K. This demonstrated agreement implies that full dielectric tuning can be expected in these ferroelectric thin films on nanosecond time scales, and also demonstrates that detrimental high-frequency nonlinear effects in device structures can be accurately predicted based on dc biased measurements.

  5. Cerenkov configuration second harmonic generation in proton-exchanged lithium niobate guides

    NASA Astrophysics Data System (ADS)

    Li, M. J.; de Micheli, M.; He, Q.; Ostrowsky, D. B.

    1990-08-01

    A theoretical and experimental study of second-harmonic generation using the Cerenkov configuration with proton-exchanged lithium niobate guides is presented. The analytic solution of the problem for the case of planar step-index guides makes it possible to identify the essential role played by the discontinuity of the nonlinear polarization at the guide-substrate interface. This leads to the prediction of an increasing conversion efficiency for decreasing values of guide nonlinearity. It is shown that the experimental results are consistent with a reduction of 50 to 70 percent of the value of the nonlinear coefficient in unannealed waveguides fabricated in slightly diluted or pure benzoic acid. The results presented permit the optimization of guide design for efficient second-harmonic generation in the Cerenkov configuration.

  6. Dynamical calculation of third-harmonic generation in a semiconductor quantum well

    NASA Astrophysics Data System (ADS)

    Guazzotti, Stefano; Pusch, Andreas; Reiter, Doris E.; Hess, Ortwin

    2016-09-01

    Nonlinear phenomena in optically excited semiconductor structures are of high interest. Here we develop a model capable of studying the dynamics of the photoexcited carriers, including Coulomb interaction on a Hartree-Fock level, on the same footing as the dynamics of the light field impinging on an arbitrary photonic structure. Applying this method to calculate the third-harmonic generation in a semiconductor quantum well embedded in a Bragg mirror structure, we find that the power-law exponent of the intensity dependence of the third-harmonic generation depends on the frequency of the exciting pulse. Off-resonant pulses follow the expected cubic dependence, while the exponent is smaller for resonant pulses due to saturation effects in the induced carrier density. Our study provides a detailed understanding of the carrier and light field dynamics during nonlinear processes.

  7. Optimal control of attosecond pulse synthesis from high-order harmonic generation

    SciTech Connect

    Ben Haj Yedder, A.; Le Bris, C.; Atabek, O.; Chelkowski, S.; Bandrauk, A. D.

    2004-04-01

    Numerical solutions of the time-dependent Schroedinger equation for a three-dimensional H atom and an efficient genetic algorithm are used to optimize short intense excitation laser pulses in order to generate high-order harmonics from which we synthesize single attosecond pulses. It is shown that chirping of excitation pulses at intensities {approx}10{sup 14} W/cm{sup 2} and duration of up to {approx}16 fs can lead to synthesis of single attosecond pulses. The optimal excitation pulses and the phases of the generated harmonics are compared with the nonoptimized ones, showing thus the usefulness of genetic algorithm schemes in the search of optimal conditions for synthesizing single attosecond pulses.

  8. Determination of chronological aging parameters in epidermal keratinocytes by in vivo harmonic generation microscopy

    PubMed Central

    Liao, Yi-Hua; Chen, Szu-Yu; Chou, Sin-Yo; Wang, Pei-Hsun; Tsai, Ming-Rung; Sun, Chi-Kuang

    2012-01-01

    Skin aging is an important issue in geriatric and cosmetic dermatology. To quantitatively analyze changes in keratinocytes related to intrinsic aging, we exploited a 1230 nm-based in vivo harmonic generation microscopy, combining second- and third-harmonic generation modalities. 52 individuals (21 men and 31 women, age range 19–79) were examined on the sun-protected volar forearm. Through quantitative analysis by the standard algorithm provided, we found that the cellular and nuclear size of basal keratinocytes, but not that of granular cells, was significantly increased with advancing age. The cellular and nuclear areas, which have an increase of 0.51 μm2 and 0.15 μm2 per year, respectively, can serve as scoring indices for intrinsic skin aging. PMID:23304649

  9. Second harmonic generation from metamaterials strongly coupled to intersubband transitions in quantum wells

    SciTech Connect

    Campione, Salvatore; Benz, Alexander; Brener, Igal; Sinclair, Michael B.; Capolino, Filippo

    2014-03-31

    We theoretically analyze the second harmonic generation capacity of two-dimensional periodic metamaterials comprising sub-wavelength resonators strongly coupled to intersubband transitions in quantum wells (QWs) at mid-infrared frequencies. The metamaterial is designed to support a fundamental resonance at ∼30 THz and an orthogonally polarized resonance at the second harmonic frequency (∼60 THz), while the asymmetric quantum well structure is designed to provide a large second order susceptibility. Upon continuous wave illumination at the fundamental frequency we observe second harmonic signals in both the forward and backward directions, with the forward efficiency being larger. We calculate the overall second harmonic conversion efficiency of the forward wave to be ∼1.3 × 10{sup −2} W/W{sup 2}—a remarkably large value, given the deep sub-wavelength dimensions of the QW structure (about 1/15th of the free space wavelength of 10 μm). The results shown in this Letter provide a strategy for designing easily fabricated sources across the entire infrared spectrum through proper choice of QW and resonator designs.

  10. High conversion efficiency pumped-cavity second harmonic generation of a diode laser

    SciTech Connect

    Keicher, D.M.

    1994-01-01

    To investigate the feasibility of producing a compact, efficient blue laser source, pumped-cavity second harmonic generation of diode lasers was explored. It is desirable to have such lasers to increase optical disk storage density, for color displays and for under-the-sea green-blue optical signal transmission. Based on assumed cavity losses, a cavity was designed and numerical analysis predicted an overall conversion efficiency to the second harmonic wavelength of 76% from a 75 mW diode laser. The diode laser used in these experiments had a single longitudinal and a single transverse mode output at 860 nm. The best conversion efficiency obtained (26%) was less than optimum due to the 2.5% single-pass linear losses associated with the cavity. However, calculations based on these higher losses are in good agreement with the experimentally determined values. In additions, a factor of 1.65 increase in the second harmonic output power is anticipated by reducing the input mirror reflectivity to better impedance-match the cavity. With this relatively low second harmonic conversion, the power to light conversion is 7.8%.

  11. High-contrast imaging of mycobacterium tuberculosis using third-harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Kim, Bo Ram; Lee, Eungjang; Park, Seung-Han

    2015-07-01

    Nonlinear optical microcopy has become an important tool in investigating biomaterials due to its various advantages such as label-free imaging capabilities. In particular, it has been shown that third-harmonic generation (THG) signals can be produced at interfaces between an aqueous medium (e.g. cytoplasm, interstitial fluid) and a mineralized lipidic surface. In this work, we have demonstrated that label-free high-contrast THG images of the mycobacterium tuberculosis can be obtained using THG microscopy.

  12. In vivo polarization dependant Second and Third harmonic generation imaging of Caenorhabditis elegans pharyngeal muscles

    NASA Astrophysics Data System (ADS)

    Filippidis, G.; Troulinaki, K.; Fotakis, C.; Tavernarakis, N.

    2009-07-01

    In this study Second and Third harmonic generation (SHG-THG) imaging measurements were performed to the pharyngeal muscles of the nematode Caenorhabditis elegans, in vivo with linearly polarized laser beam. Complementary information about the anatomy of the pharynx and the morphology of the anterior part of the worm were extracted. THG signals proved to have no dependence on incident light polarization, while SHG images are highly sensitive to the changes of the incident linearly polarized light.

  13. Second harmonic generation in periodically poled lithium niobate waveguide using femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Zhang, Shuanggen; Yao, Jianghong; Fan, Yaxian; Liu, Weiwei; Liu, Yange; Shi, Qing; Huang, Zhangchao; Lu, Fuyun

    2008-11-01

    We present in this paper the fabrication and characterization of thermally stable double line waveguides in Z-cut periodically poled Lithium Niobate crystals. The waveguides were fabricated by using a femto-second laser, and utilized for second-harmonic generation. Our experiments have shown that a quasi-phase matching wavelength of 1548.2 nm, a tuning bandwidth of 2 nm, and a tuning temperature range of 150.4+/-1.6°C can be achieved.

  14. Second harmonic generation imaging of dermal collagen component in human keloid tissue

    NASA Astrophysics Data System (ADS)

    Yu, H. B.; Chen, S.; Zhu, X. Q.; Yang, H. Q.; Chen, J. X.

    2011-01-01

    In this paper, we report second harmonic generation (SHG) imaging of human keloid tissue. High resolution SHG images of collagen component were obtained in the superficial, medial and deep dermis of human keloid tissue, respectively. Our results show that this method has a capability to observe the structure of collagen component in human keloid tissue, which will help to better understand the formation process of human keloid scar at the molecular level.

  15. Recollision dynamics of electron wave packets in high-order harmonic generation

    NASA Astrophysics Data System (ADS)

    Yuan, Kai-Jun; Bandrauk, André D.

    2009-11-01

    We numerically investigate the dynamics of recollision of an electron in high-order harmonic generation (HHG) for an H atom and a molecular ion H2+ using a short (ten optical cycles), and intense (I0≥1014W/cm2) , z -polarized linear laser pulse with wavelength 800 nm by accurately solving the three-dimensional time-dependent Schrödinger equation. A time-frequency analysis obtained via Gabor transforms is employed to identify electron recollision and recombination times responsible for the generation of harmonics. We find that the HHG spectra are mainly attributed to the recollision of an inner electron wave packet with the parent ion in agreement with the classical recollision model. A time delay of the electron recollision occurs between wave packets in inner and outer regions, near to and far from the parent ion, due to different phase of the acceleration (as well as dipole velocity) of the electron. Inner wave packets at recollision contain mainly short and long trajectories whereas outer wave packets contain only single trajectories. Lower-order harmonics are generated mainly by single recollisions near field extrema, i.e., in strong electric fields whereas higher-order harmonics are generated by double trajectories with different intensities. In the case of H2+ at a critical nuclear distance for charge resonance enhanced ionization, we also find that HHG mainly comes from contributions of the inner electron wave packet, but with more complex recollision trajectories due to the presence of more than one Coulomb center. Triple recollision trajectories are shown to occur generally for the latter.

  16. Optical second-harmonic generation enhanced by a twist defect in ferroelectric liquid crystals.

    PubMed

    Hoshi, Hajime; Ishikawa, Ken; Takezoe, Hideo

    2003-08-01

    Second-harmonic generation (SHG) spectra were numerically calculated in ferroelectric liquid crystals with a twist defect. It is shown that SHG is enhanced when the SHG wavelength is close to the defect mode. The spectral width of the enhanced peak becomes sharper with increasing the sample thickness at the same rate for the width of the defect mode peak. The SHG peak intensity increases with about seventh power of the sample thickness.

  17. Periodically poled LiNbO3 ridge waveguides on silicon for second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Chauvet, Mathieu; Henrot, Fabien; Gauthier-Manuel, Ludovic; Devaux, Fabrice; Pêcheur, Vincent; Maillotte, Hervé; Bassignot, Florent; Dahmani, Brahim

    2016-05-01

    Nonlinear periodically poled ridge LiNbO3 waveguides have been fabricated on silicon substrates. Components are micromachined with a precision dicing machine and/or by grinding or polishing steps. They show efficient second harmonic generation at telecommunication wavelengths with normalized conversion reaching 600%/W in a 20mm long device. Influence of geometrical non uniformities of waveguides due to fabrication process is asserted. Components characteristics are studied notably their robustness and tunability versus temperature.

  18. Second harmonic generation in a low-loss orientation-patterned GaAs waveguide.

    PubMed

    Fedorova, K A; McRobbie, A D; Sokolovskii, G S; Schunemann, P G; Rafailov, E U

    2013-07-15

    The technology of low-loss orientation-patterned gallium arsenide (OP-GaAs) waveguided crystals was developed and realized by reduction of diffraction scattering on the waveguide pattern. The propagation losses in the OP-GaAs waveguide were estimated to be as low as 2.1 dB/cm, thus demonstrating the efficient second harmonic generation at 1621 nm under an external pumping.

  19. Theory of second-harmonic generation of molecular systems: The steady-state case

    SciTech Connect

    Lin, S.H.; Alden, R.G. ); Villaeys, A.A.; Pflumio, V. )

    1993-10-01

    In this paper, a general formalism for treating both steady-state and time-resolved second-harmonic generation for molecular systems is presented. Here, only the steady-state case will be reported. The adiabatic approximation is introduced. Four important cases, resonance-resonance, resonance--off-resonance, off-resonance--resonance, and off-resonance--off-resonance transitions, have been considered. Finally, numerical calculations of rhodamine 6G are performed to demonstrate the applications of theoretical results.

  20. Multiphoton ionization and third-harmonic generation in atoms and molecules

    SciTech Connect

    Compton, R.N.

    1982-01-01

    Resonantly enhanced multiphoton ionization (REMPI) provides a powerful new method for investigating atomic and molecular energy levels. The method is particularly useful in discovering and characterizing certain optically forbidden transitions. The method is particularly well suited for studying Rydberg transitions in molecules and is experimentally easier than the traditional use of far ultraviolet radiation in conventional spectroscopy. Research on multiphoton ionization and third-harmonic generation is reviewed. (WHK)

  1. Diffractive imaging using a polychromatic high-harmonic generation soft-x-ray source

    NASA Astrophysics Data System (ADS)

    Dilanian, Ruben A.; Chen, Bo; Williams, Garth J.; Quiney, Harry M.; Nugent, Keith A.; Teichmann, Sven; Hannaford, Peter; Dao, Lap V.; Peele, Andrew G.

    2009-07-01

    A new approach to diffractive imaging using polychromatic diffraction data is described. The method is tested using simulated and experimental data and is shown to yield high-quality reconstructions. Diffraction data produced using a high-harmonic generation source are considered explicitly here. The formalism can be readily adapted, however, to any short-wavelength source producing a discrete spectrum and possessing sufficient spatial coherence.

  2. Enhanced second-harmonic generation driven from magnetic dipole resonance in AlGaAs nanoantennas

    NASA Astrophysics Data System (ADS)

    Carletti, Luca; Rocco, Davide; Locatelli, Andrea; Gili, Valerio; Leo, Giuseppe; De Angelis, Costantino

    2016-04-01

    We model the linear and nonlinear optical response of disk-shaped AlGaAs nanoantennas. We design nanoantennas with a magnetic dipole resonant mode in the near-infrared wavelength range, and we analyze volume second-harmonic generation driven by a magnetic dipole resonance by predicting a conversion efficiency exceeding 10-3 with 1 GW/cm2 of pump intensity.

  3. Quasi-phase matching and quantum control of high harmonic generation in waveguides using counterpropagating beams

    DOEpatents

    Zhang, Xiaoshi; Lytle, Amy L.; Cohen, Oren; Kapteyn, Henry C.; Murnane, Margaret M.

    2010-11-09

    All-optical quasi-phase matching (QPM) uses a train of counterpropagating pulses to enhance high-order harmonic generation (HHG) in a hollow waveguide. A pump pulse enters one end of the waveguide, and causes HHG in the waveguide. The counterpropagation pulses enter the other end of the waveguide and interact with the pump pulses to cause QPM within the waveguide, enhancing the HHG.

  4. Frequency-resolved optical-gating measurements of ultrashort pulses using surface third-harmonic generation

    SciTech Connect

    Tsang, T.; Krumbuegel, M.A.; DeLong, K.W.; Fittinghoff, D.N.; Trebino, R.

    1996-09-01

    We demonstrate what is to our knowledge the first frequency-resolved optical gating (FROG) technique to measure ultrashort pulses from an unamplified Ti:sapphire laser oscillator without direction-of-time ambiguity. This technique utilizes surface third-harmonic generation as the nonlinear-optical effect and, surprisingly, is the most sensitive third-order FROG geometry yet. {copyright} {ital 1996 Optical Society of America.}

  5. High-order harmonic generation by chirped and self-guided femtosecond laser pulses. II. Time-frequency analysis

    SciTech Connect

    Tosa, V.; Kim, H.T.; Kim, I.J.; Nam, C.H.

    2005-06-15

    We present a time-dependent analysis of high-order harmonics generated by a self-guided femtosecond laser pulse propagating through a long gas jet. A three-dimensional model is used to calculate the harmonic fields generated by laser pulses, which only differ by the sign of their initial chirp. The time-frequency distributions of the single-atom dipole and harmonic field reveal the dynamics of harmonic generation in the cutoff. A time-dependent phase-matching calculation was performed, taking into account the self-phase modulation of the laser field. Good phase matching holds for only few optical cycles, being dependent on the electron trajectory. When the cutoff trajectory is phase matched, emitted harmonics are locked in phase and the emission intensity is maximized.

  6. Impact of electron ionization on the generation of high-order harmonics from molecules

    SciTech Connect

    Brener, S.; Moiseyev, N.; Ivanov, M. V.

    2003-08-01

    When the laser frequency is tuned to be equal to the molecular electronic excitation, high-order harmonics are generated due to the electronic dipole transitions between the corresponding two potential-energy surfaces (PES). A natural, often taken, choice is the PES of the field-free molecular system. In this special choice the ionization phenomenon is not considered. Only the effect of the dissociation is considered. The method we developed enables one to remain within the framework of the 2-PES approximation and yet to include also the ionization effect in the calculations of molecular high-order harmonic generation spectra. In this approach the coupling between the electronic and nuclear motions is taken into consideration by using coupled complex adiabatic PES. As an illustrative numerical example, we calculated the high harmonic generation (HHG) spectra of H{sub 2}{sup +} in a 730-nm laser with the intensity of 8.77x10{sup 13} W/cm{sup 2}. The inclusion of the ionization in our approach not only enables the electrons to tunnel through the effective static potential barrier, but also apply an asymmetric force which accelerates the electron before ionization takes place. Therefore, indirectly the inclusion of the ionization by the laser field may lead eventually to an enhanced HHG spectra in comparison with the calculated one when the ''natural'' choice of the field-free 2PES is taken.

  7. Generation of tunable ultrafast ultraviolet third harmonic by collinear compensation of group-velocity mismatch

    NASA Astrophysics Data System (ADS)

    Meng, Xianghao; Liu, Huagang; Huang, Jianhong; Wu, Hongchun; Deng, Jing; Dai, Shutao; Weng, Wen; Lin, Wenxiong

    2015-10-01

    We demonstrate a high efficient frequency tripling configuration of Ti: sapphire amplifier system for wavelength-tunable ultrafast ultraviolet laser generation. A new nonlinear crystal Ba1-xB2-y-zO4SixAlyGaz and a type-II phase-matched β-BaB2O4 crystal are employed for the second and the third harmonic generation, respectively. Significant improvement in conversion efficiency of frequency tripling is achieved by using a 65°-cut, 3-mm-long β-BaB2O4 crystal as the collinear group velocity compensation plate. Tunable ultraviolet pulse within the wavelength range from 256.7 to 276.7 nm have been produced, with a maximum average power of 212 mW, corresponding to a conversion efficiency of 8.48% for the third harmonic generation with 2.5 W fundamental power. The maximum pulse energy of the third harmonic is up to 0.21 mJ and it is estimated that the peak power is above 1 GW at 266.7 nm.

  8. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    SciTech Connect

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; Tarazkar, Maryam; Romanov, Dmitri A.; Levis, Robert J.; Gaffney, Jim A.; Foord, Mark; Libby, Stephen B.; Jaron-Becker, Agnieskzka; Becker, Andreas; Plaja, Luis; Muranane, Margaret M.; Kapteyn, Henry C.; Popmintchev, Tenio

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams in the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.

  9. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    DOE PAGES

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; et al

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams inmore » the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.« less

  10. Correspondence of below-threshold high-order-harmonic generation and frustrated tunneling ionization

    NASA Astrophysics Data System (ADS)

    Xiong, Wei-Hao; Xiao, Xiang-Ru; Peng, Liang-You; Gong, Qihuang

    2016-07-01

    Among many of the nonlinear phenomena induced by strong laser pulses, two of the important processes are the harmonic generation and the creation of neutral atoms in the Rydberg states. We carry out a joint study of the below-threshold high-order-harmonic (BTH) generation and the production of low-lying Rydberg atoms driven by an intense few-cycle midinfrared laser pulse. Our results are based on the numerical solution to the three-dimensional time-dependent Schrödinger equation within the single active electron approximation and a semiclassical simulation. The yields of BTH and low-lying Rydberg atoms are found to have a similar carrier envelope phase dependence. We find that both processes can be faithfully described semiclassically in the deep tunneling regime. The trajectory analysis shows that these two processes share the same series of trajectories and can be simultaneously manipulated by the driving pulse shape. Our finding bridges the below-threshold high-order-harmonic generation and the frustrated tunneling ionization.

  11. Background-free electric field-induced second harmonic generation with interdigitated combs of electrodes.

    PubMed

    Jašinskas, Vidmantas; Gedvilas, Mindaugas; Račiukaitis, Gediminas; Gulbinas, Vidmantas

    2016-06-15

    The electric field-induced second harmonic (EFISH) generation is a powerful tool for the investigation of optical nonlinearities, material polarization, internal electric fields, and other properties of photonic materials and devices. A conventional generation of the second harmonics (SH) in materials with the disturbed centrosymmetry causes a field-independent background to EFISH and limits its applications. Here we suggest and analyze the application of the interdigitated combs of electrodes for EFISH generation in thin films. Interdigitated electrodes form an optical transmission amplitude diffraction grating. Phase matching of the EFISH radiation creates unusual diffraction fringes with the zero intensity along the zeroth order direction and with the diffraction angles different from diffraction angles of incident fundamental laser radiation and its second harmonics. It enables a simple geometrical separation of the EFISH signal from a conventional SH background, simplifies the sample preparation, and provides additional experimental possibilities. We demonstrate applicability of the suggested technique for characterization of submicrometer thickness organic films of transparent and resonantly interacting polymers and of their mixtures. PMID:27304282

  12. Second harmonic generation by propagation of a p-polarized obliquely incident laser beam in underdense plasma

    SciTech Connect

    Jha, Pallavi; Agrawal, Ekta

    2014-05-15

    An analytical study of second harmonic generation due to interaction an intense, p-polarized laser beam propagating obliquely in homogeneous underdense plasma, in the mildly relativistic regime, has been presented. The efficiency of the second harmonic radiation as well as its detuning length has been obtained and their variation with the angle of incidence is analyzed. It is shown that, for a given plasma electron density, the second harmonic efficiency increases with the angle of incidence while the detuning length decreases. The second harmonic amplitude vanishes at normal incidence of the laser beam.

  13. First Demonstration of the Echo-Enabled Harmonic Generation Technique for Short-Wavelength Seeded Free Electron Lasers

    SciTech Connect

    Xiang, D.; Colby, E.; Dunning, M.; Gilevich, S.; Hast, C.; Jobe, K.; McCormick, D.; Nelson, J.; Raubenheimer, T.O.; Soong, K.; Stupakov, G.; Szalata, Z.; Walz, D.; Weathersby, S.; Woodley, M.; Pernet, P.-L.; /Ecole Polytechnique, Lausanne

    2010-08-25

    We report the first experimental demonstration of the echo-enabled harmonic generation (EEHG) technique which holds great promise for generation of high power, fully coherent short-wavelength radiation. In this experiment, coherent radiation at the 3rd and 4th harmonic of the second seed laser is generated from the so-called beam echo effect. The experiment confirms the physics behind this technique and paves the way for applying the EEHG technique for seeded x-ray free electron lasers.

  14. X-ray spectral diagnostics of laser harmonic generation in the interaction of relativistic femtosecond laser pulses with clusters

    NASA Astrophysics Data System (ADS)

    Faenov, A. Ya; Oks, E.; Dalimier, E.; Skobelev, I. Yu; Pikuz, S. A.; Pikuz, T. A.; Zhvaniya, I. A.; Fukuda, Y.; Andreev, A.; Koga, J.; Sakaki, H.; Kotaki, H.; Pirozhkov, A. S.; Hayashi, Y.; Kawachi, T.; Kando, M.; Kondo, K.; Zhidkov, A. G.; Kodama, R.

    2016-04-01

    It is shown that the production of X-ray emission spectra in the interaction of high-intensity laser radiation with cluster targets may be affected by the bichromatic oscillating electric field arising from the generation of the second harmonic of laser radiation. A technique is proposed for diagnosing harmonic generation in laser - cluster interactions using the spectral line profiles of multiply charged helium ions. The efficiency of second harmonic generation at a laser intensity of 3 × 1018 W cm-2 is shown to amount to about 2%.

  15. Enhanced high-order-harmonic generation and wave mixing via two-color multiphoton excitation of atoms and molecules

    NASA Astrophysics Data System (ADS)

    Avetissian, H. K.; Avchyan, B. R.; Mkrtchian, G. F.

    2016-07-01

    We consider harmonics generation and wave mixing by two-color multiphoton resonant excitation of three-level atoms and molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is investigated. The obtained analytical results on the basis of a generalized rotating wave approximation are in a good agreement with numerical calculations. The results applied to the hydrogen atoms and homonuclear diatomic molecular ions show that one can achieve efficient generation of moderately high multicolor harmonics via multiphoton resonant excitation by appropriate laser pulses.

  16. Life Cycle Greenhouse Gas Emissions of Coal-Fired Electricity Generation: Systematic Review and Harmonization

    SciTech Connect

    Whitaker, M.; Heath, G. A.; O'Donoughue, P.; Vorum, M.

    2012-04-01

    This systematic review and harmonization of life cycle assessments (LCAs) of utility-scale coal-fired electricity generation systems focuses on reducing variability and clarifying central tendencies in estimates of life cycle greenhouse gas (GHG) emissions. Screening 270 references for quality LCA methods, transparency, and completeness yielded 53 that reported 164 estimates of life cycle GHG emissions. These estimates for subcritical pulverized, integrated gasification combined cycle, fluidized bed, and supercritical pulverized coal combustion technologies vary from 675 to 1,689 grams CO{sub 2}-equivalent per kilowatt-hour (g CO{sub 2}-eq/kWh) (interquartile range [IQR]= 890-1,130 g CO{sub 2}-eq/kWh; median = 1,001) leading to confusion over reasonable estimates of life cycle GHG emissions from coal-fired electricity generation. By adjusting published estimates to common gross system boundaries and consistent values for key operational input parameters (most importantly, combustion carbon dioxide emission factor [CEF]), the meta-analytical process called harmonization clarifies the existing literature in ways useful for decision makers and analysts by significantly reducing the variability of estimates ({approx}53% in IQR magnitude) while maintaining a nearly constant central tendency ({approx}2.2% in median). Life cycle GHG emissions of a specific power plant depend on many factors and can differ from the generic estimates generated by the harmonization approach, but the tightness of distribution of harmonized estimates across several key coal combustion technologies implies, for some purposes, first-order estimates of life cycle GHG emissions could be based on knowledge of the technology type, coal mine emissions, thermal efficiency, and CEF alone without requiring full LCAs. Areas where new research is necessary to ensure accuracy are also discussed.

  17. High-Gain High-Field Fusion Plasma

    PubMed Central

    Li, Ge

    2015-01-01

    A Faraday wheel (FW)—an electric generator of constant electrical polarity that produces huge currents—could be implemented in an existing tokamak to study high-gain high-field (HGHF) fusion plasma, such as the Experimental Advanced Superconducting Tokamak (EAST). HGHF plasma can be realized in EAST by updating its pulsed-power system to compress plasma in two steps by induction fields; high gains of the Lawson trinity parameter and fusion power are both predicted by formulating the HGHF plasma. Both gain rates are faster than the decrease rate of the plasma volume. The formulation is checked by earlier ATC tests. Good agreement between theory and tests indicates that scaling to over 10 T at EAST may be possible by two-step compressions with a compression ratio of the minor radius of up to 3. These results point to a quick new path of fusion plasma study, i.e., simulating the Sun by EAST. PMID:26507314

  18. Compensation for Harmonic Currents and Reactive Power in Wind Power Generation System using PWM Inverter

    NASA Astrophysics Data System (ADS)

    Shinohara, Katsuji; Shinhatsubo, Kurato; Iimori, Kenichi; Yamamoto, Kichiro; Saruban, Takamichi; Yamaemori, Takahiro

    In recent year, consciousness of environmental problems is enhancing, and the price of the electric power purchased by an electric power company is established expensive for the power plant utilizing the natural energy. So, the introduction of the wind power generation is promoted in Japan. Generally, squirrel-cage induction machines are widely used as a generator in wind power generation system because of its small size, lightweight and low-cost. However, the induction machines do not have a source of excitation. Thus, it causes the inrush currents and the instantaneous voltage drop when the generator is directly connected to a power grid. To reduce the inrush currents, an AC power regulator is used. Wind power generations are frequently connected to and disconnected from the power grid. However, when the inrush currents are reduced, harmonic currents are caused by phase control of the AC power regulator. And the phase control of AC power regulator cannot control the power factor. Therefore, we propose the use of the AC power regulator to compensate for the harmonic currents and reactive power in the wind power generation system, and demonstrate the validity of its system by simulated and experimental results.

  19. Ablation of boron carbide for high-order harmonic generation of ultrafast pulses in laser-produced plasma

    NASA Astrophysics Data System (ADS)

    Ganeev, R. A.; Suzuki, M.; Kuroda, H.

    2016-07-01

    We demonstrate the generation of harmonics up to the 27th order (λ=29.9 nm) of 806 nm radiation in the boron carbide plasma. We analyze the advantages and disadvantages of this target compared with the ingredients comprising B4C (solid boron and graphite) by studying the plasma emission and harmonic spectra from three species. We compare different schemes of the two-color pump of B4C plasma, particularly using the second harmonics of 806 nm laser and optical parametric amplifier (1310 nm) as the assistant fields, as well as demonstrate the sum and difference frequency generation using the mixture of the wavelengths of two laser sources. These studies showed the advantages of the two-color pump of B4C plasma leading to the stable harmonic generation and the growth of harmonic conversion efficiency. We also show that the coincidence of harmonic and plasma emission wavelengths in most cases does not cause the enhancement or decrease of the conversion efficiency of this harmonic. Our spatial characterization of harmonics shows their on-axis modification depending on the conditions of frequency conversion.

  20. Enhanced Third Harmonic Generation in Single Germanium Nanodisks Excited at the Anapole Mode.

    PubMed

    Grinblat, Gustavo; Li, Yi; Nielsen, Michael P; Oulton, Rupert F; Maier, Stefan A

    2016-07-13

    We present an all-dielectric germanium nanosystem exhibiting a strong third order nonlinear response and efficient third harmonic generation in the optical regime. A thin germanium nanodisk shows a pronounced valley in its scattering cross section at the dark anapole mode, while the electric field energy inside the disk is maximized due to high confinement within the dielectric. We investigate the dependence of the third harmonic signal on disk size and pump wavelength to reveal the nature of the anapole mode. Each germanium nanodisk generates a high effective third order susceptibility of χ((3)) = 4.3 × 10(-9) esu, corresponding to an associated third harmonic conversion efficiency of 0.0001% at an excitation wavelength of 1650 nm, which is 4 orders of magnitude greater than the case of an unstructured germanium reference film. Furthermore, the nonlinear conversion via the anapole mode outperforms that via the radiative dipolar resonances by about 1 order of magnitude, which is consistent with our numerical simulations. These findings open new possibilities for the optimization of upconversion processes on the nanoscale through the appropriate engineering of suitable dielectric materials.

  1. The Interplay of Symmetry and Scattering Phase in Second Harmonic Generation from Gold Nanoantennas.

    PubMed

    Gennaro, Sylvain D; Rahmani, Mohsen; Giannini, Vincenzo; Aouani, Heykel; Sidiropoulos, Themistoklis P H; Navarro-Cía, Miguel; Maier, Stefan A; Oulton, Rupert F

    2016-08-10

    Nonlinear phenomena are central to modern photonics but, being inherently weak, typically require gradual accumulation over several millimeters. For example, second harmonic generation (SHG) is typically achieved in thick transparent nonlinear crystals by phase-matching energy exchange between light at initial, ω, and final, 2ω, frequencies. Recently, metamaterials imbued with artificial nonlinearity from their constituent nanoantennas have generated excitement by opening the possibility of wavelength-scale nonlinear optics. However, the selection rules of SHG typically prevent dipole emission from simple nanoantennas, which has led to much discussion concerning the best geometries, for example, those breaking centro-symmetry or incorporating resonances at multiple harmonics. In this work, we explore the use of both nanoantenna symmetry and multiple harmonics to control the strength, polarization and radiation pattern of SHG from a variety of antenna configurations incorporating simple resonant elements tuned to light at both ω and 2ω. We use a microscopic description of the scattering strength and phases of these constituent particles, determined by their relative positions, to accurately predict the SHG radiation observed in our experiments. We find that the 2ω particles radiate dipolar SHG by near-field coupling to the ω particle, which radiates SHG as a quadrupole. Consequently, strong linearly polarized dipolar SHG is only possible for noncentro-symmetric antennas that also minimize interference between their dipolar and quadrupolar responses. Metamaterials with such intra-antenna phase and polarization control could enable compact nonlinear photonic nanotechnologies.

  2. The Interplay of Symmetry and Scattering Phase in Second Harmonic Generation from Gold Nanoantennas.

    PubMed

    Gennaro, Sylvain D; Rahmani, Mohsen; Giannini, Vincenzo; Aouani, Heykel; Sidiropoulos, Themistoklis P H; Navarro-Cía, Miguel; Maier, Stefan A; Oulton, Rupert F

    2016-08-10

    Nonlinear phenomena are central to modern photonics but, being inherently weak, typically require gradual accumulation over several millimeters. For example, second harmonic generation (SHG) is typically achieved in thick transparent nonlinear crystals by phase-matching energy exchange between light at initial, ω, and final, 2ω, frequencies. Recently, metamaterials imbued with artificial nonlinearity from their constituent nanoantennas have generated excitement by opening the possibility of wavelength-scale nonlinear optics. However, the selection rules of SHG typically prevent dipole emission from simple nanoantennas, which has led to much discussion concerning the best geometries, for example, those breaking centro-symmetry or incorporating resonances at multiple harmonics. In this work, we explore the use of both nanoantenna symmetry and multiple harmonics to control the strength, polarization and radiation pattern of SHG from a variety of antenna configurations incorporating simple resonant elements tuned to light at both ω and 2ω. We use a microscopic description of the scattering strength and phases of these constituent particles, determined by their relative positions, to accurately predict the SHG radiation observed in our experiments. We find that the 2ω particles radiate dipolar SHG by near-field coupling to the ω particle, which radiates SHG as a quadrupole. Consequently, strong linearly polarized dipolar SHG is only possible for noncentro-symmetric antennas that also minimize interference between their dipolar and quadrupolar responses. Metamaterials with such intra-antenna phase and polarization control could enable compact nonlinear photonic nanotechnologies. PMID:27433989

  3. Enhanced Third Harmonic Generation in Single Germanium Nanodisks Excited at the Anapole Mode.

    PubMed

    Grinblat, Gustavo; Li, Yi; Nielsen, Michael P; Oulton, Rupert F; Maier, Stefan A

    2016-07-13

    We present an all-dielectric germanium nanosystem exhibiting a strong third order nonlinear response and efficient third harmonic generation in the optical regime. A thin germanium nanodisk shows a pronounced valley in its scattering cross section at the dark anapole mode, while the electric field energy inside the disk is maximized due to high confinement within the dielectric. We investigate the dependence of the third harmonic signal on disk size and pump wavelength to reveal the nature of the anapole mode. Each germanium nanodisk generates a high effective third order susceptibility of χ((3)) = 4.3 × 10(-9) esu, corresponding to an associated third harmonic conversion efficiency of 0.0001% at an excitation wavelength of 1650 nm, which is 4 orders of magnitude greater than the case of an unstructured germanium reference film. Furthermore, the nonlinear conversion via the anapole mode outperforms that via the radiative dipolar resonances by about 1 order of magnitude, which is consistent with our numerical simulations. These findings open new possibilities for the optimization of upconversion processes on the nanoscale through the appropriate engineering of suitable dielectric materials. PMID:27331867

  4. Temperature dependence of acoustic harmonics generated by nonlinear ultrasound wave propagation in water at various frequencies.

    PubMed

    Maraghechi, Borna; Hasani, Mojtaba H; Kolios, Michael C; Tavakkoli, Jahan

    2016-05-01

    Ultrasound-based thermometry requires a temperature-sensitive acoustic parameter that can be used to estimate the temperature by tracking changes in that parameter during heating. The objective of this study is to investigate the temperature dependence of acoustic harmonics generated by nonlinear ultrasound wave propagation in water at various pulse transmit frequencies from 1 to 20 MHz. Simulations were conducted using an expanded form of the Khokhlov-Zabolotskaya-Kuznetsov nonlinear acoustic wave propagation model in which temperature dependence of the medium parameters was included. Measurements were performed using single-element transducers at two different transmit frequencies of 3.3 and 13 MHz which are within the range of frequencies simulated. The acoustic pressure signals were measured by a calibrated needle hydrophone along the axes of the transducers. The water temperature was uniformly increased from 26 °C to 46 °C in increments of 5 °C. The results show that the temperature dependence of the harmonic generation is different at various frequencies which is due to the interplay between the mechanisms of absorption, nonlinearity, and focusing gain. At the transmit frequencies of 1 and 3.3 MHz, the harmonic amplitudes decrease with increasing the temperature, while the opposite temperature dependence is observed at 13 and 20 MHz. PMID:27250143

  5. An azo-bridged ferroelectric liquid crystal with highly enhanced second and third harmonic generation.

    PubMed

    Zhang, Yongqiang; Ortega, Josu; Baumeister, Ute; Folcia, César L; Sanz-Enguita, Gerardo; Walker, Christopher; Rodriguez-Conde, Sofía; Etxebarria, Jesus; O'Callaghan, Michael J; More, Kundalika

    2012-10-01

    A laterally azo-bridged trimer ferroelectric liquid crystal (FLC) incorporating a strong chromophore along its polar axis was synthesized and characterized by polarized-light optical microscopy, differential scanning calorimetry, two-dimensional X-ray diffraction analysis, electro-optical measurements, and nonlinear optical (NLO) investigations. This mesogen exhibits a thermodynamically stable enantiotropic SmC* phase and a bistable ferroelectric switching in a surface stabilized cell with bookshelf geometry. It gives the resonance-enhanced d(22) coefficient of 28 pm V(-1) (λ = 1.369 μm) for second harmonic generation (SHG), the largest NLO susceptibility reported to date for all FLCs. At the same wavelength, a new type of helicoidal phase matching assisted by the helical SmC* structure was identified. When the second harmonic wavelength of 780 nm is far away from the resonance wavelength (λ(max) = 572 nm), the d(22) coefficient is reduced to 6.8 pm V(-1) (λ = 1.56 μm). In addition to a strong SHG activity, the trimer also shows a strong third harmonic generation (THG) with an estimated third-order nonlinear susceptibility of χ((3)) = ~3 × 10(-11) esu (λ = 1.56 μm), among the largest χ((3)) value reported from THG measurements for liquid crystals. This work enables viable applications of FLCs in nonlinear optics and offers an innovative approach to develop new FLCs with larger NLO strength. PMID:22909407

  6. Third-harmonic generation enhancement in polymer-dispersed liquid crystal grating

    NASA Astrophysics Data System (ADS)

    Wicharn, S.; Buranasiri, P.

    2014-09-01

    In this paper, the enhancement of third-harmonic generation in one-dimensional periodic grating structure with lowindex contrast, which is produced by holographic illuminated liquid crystal droplets and called polymer-dispersed liquid crystal grating, with near-infrared pumping has been demonstrated. The observed enhancement process is theoretically explained and modeled with a multi-scale perturbation analysis and split-step Fourier transform technique, respectively. We show that the third-harmonic generation has been enhanced by setting the fundamental frequency wavelength to the long-wavelength band-edge of the first photonic band-gap of this periodic structure and satisfying band-edge phasematched condition. The numerical results show that a dramatic enhancement of the third-harmonic field is observed near the long-wavelength band-edge of the second photonic band-gap. Furthermore, the conversion efficiency of thirdharmonic field of forward-propagating direction is more than of backward-propagating direction by a factor of 600.

  7. Advanced properties of extended plasmas for efficient high-order harmonic generation

    SciTech Connect

    Ganeev, R. A.; Suzuki, M.; Kuroda, H.

    2014-05-15

    We demonstrate the advanced properties of extended plasma plumes (5 mm) for efficient harmonic generation of laser radiation compared with the short lengths of plasmas (∼0.3–0.5 mm) used in previous studies. The harmonic conversion efficiency quadratically increased with the growth of plasma length. The studies of this process along the whole extreme ultraviolet range using the long plasma jets produced on various metal surfaces, particularly including the resonance-enhanced laser frequency conversion and two-color pump, are presented. Such plasmas could be used for the quasi-phase matching experiments by proper modulation of the spatial characteristics of extended ablating area and formation of separated plasma jets.

  8. Second Harmonic Generation and Confined Acoustic Phonons in HighlyExcited Semiconductor Nanocrystals

    SciTech Connect

    Son, Dong Hee; Wittenberg, Joshua S.; Banin, Uri; Alivisatos, A.Paul

    2006-03-30

    The photo-induced enhancement of second harmonic generation, and the effect of nanocrystal shape and pump intensity on confined acoustic phonons in semiconductor nanocrystals, has been investigated with time-resolved scattering and absorption measurements. The second harmonic signal showed a sublinear increase of the second order susceptibility with respect to the pump pulse energy, indicating a reduction of the effective one-electron second-order nonlinearity with increasing electron-hole density in the nanocrystals. The coherent acoustic phonons in spherical and rod-shaped semiconductor nanocrystals were detected in a time-resolved absorption measurement. Both nanocrystal morphologies exhibited oscillatory modulation of the absorption cross section, the frequency of which corresponded to their coherent radial breathing modes. The amplitude of the oscillation also increased with the level of photoexcitation, suggesting an increase in the amplitude of the lattice displacement as well.

  9. Probing nuclear motion by frequency modulation of molecular high-order harmonic generation.

    PubMed

    Bian, Xue-Bin; Bandrauk, André D

    2014-11-01

    Molecular high-order harmonic generation (MHOHG) in a non-Born-Oppenheimer treatment of H(2)(+), D(2)(+), is investigated by numerical simulations of the corresponding time-dependent Schrödinger equations in full dimensions. As opposed to previous studies on amplitude modulation of intracycle dynamics in MHOHG, we demonstrate redshifts as frequency modulation (FM) of intercycle dynamics in MHOHG. The FM is induced by nuclear motion using intense laser pulses. Compared to fixed-nuclei approximations, the intensity of MHOHG is much higher due to the dependence of enhanced ionization on the internuclear distance. The width and symmetry of the spectrum of each harmonic in MHOHG encode rich information on the dissociation process of molecules at the rising and falling parts of the laser pulses, which can be used to retrieve the nuclear dynamics. Isotope effects are studied to confirm the FM mechanism.

  10. Temporal coherence of high-order harmonics generated at solid surfaces

    NASA Astrophysics Data System (ADS)

    Hemmers, D.; Behmke, M.; Karsch, S.; Keyling, J.; Major, Z.; Stelzmann, C.; Pretzler, G.

    2014-07-01

    We present interferometric measurements of the temporal coherence of high-order harmonics generated by reflection of a titanium sapphire laser off a solid surface. It is found that the coherence length of the harmonic emission is significantly reduced compared with the bandwidth limited case. To identify the responsible mechanism, the acquired data were analyzed by means of particle-in-cell simulations, whose results show good agreement between the calculated spectra and the measured coherence times. We show that the observed broadening can be understood consistently by the occurrence of a Doppler shift induced by the moving plasma surface, which is dented by the radiation pressure of the laser pulse. In this case, this Doppler effect would also lead to positive chirp of the emitted radiation.

  11. Generation and Detection of Higher Harmonics in Rayleigh Waves Using Laser Ultrasound

    SciTech Connect

    Herrmann, Jan; Jacobs, Laurence J.; Qu Jianmin; Kim, Jin-Yeon

    2006-03-06

    This research studies higher harmonics of Rayleigh surface waves propagating in nickel base superalloys. Rayleigh waves are used because they carry most of the energy and travel along the surface of a specimen where fatigue damage is typically initiated. The energy concentration near the free surface leads to stronger nonlinear effects compared to bulk waves. An ultrasonic piezoelectric transducer together with a plastic wedge is used for the experimental generation of the Rayleigh wave. The detection system consists of a laser heterodyne interferometer. Measurements are performed to detect the fundamental wave as well as the second harmonic. The amplitude ratio is related to the nonlinearity parameter {beta} which is typically used to describe changes in microstructure and investigate fatigue damage.

  12. Bright multi-keV harmonic generation from relativistically oscillating plasma surfaces.

    PubMed

    Dromey, B; Kar, S; Bellei, C; Carroll, D C; Clarke, R J; Green, J S; Kneip, S; Markey, K; Nagel, S R; Simpson, P T; Willingale, L; McKenna, P; Neely, D; Najmudin, Z; Krushelnick, K; Norreys, P A; Zepf, M

    2007-08-24

    The first evidence of x-ray harmonic radiation extending to 3.3 A, 3.8 keV (order n>3200) from petawatt class laser-solid interactions is presented, exhibiting relativistic limit efficiency scaling (eta approximately n{-2.5}-n{-3}) at multi-keV energies. This scaling holds up to a maximum order, n{RO} approximately 8{1/2}gamma;{3}, where gamma is the relativistic Lorentz factor, above which the first evidence of an intensity dependent efficiency rollover is observed. The coherent nature of the generated harmonics is demonstrated by the highly directional beamed emission, which for photon energy hnu>1 keV is found to be into a cone angle approximately 4 degrees , significantly less than that of the incident laser cone (20 degrees ).

  13. In-phased second harmonic wave array generation with intra-Talbot-cavity frequency-doubling.

    PubMed

    Hirosawa, Kenichi; Shohda, Fumio; Yanagisawa, Takayuki; Kannari, Fumihiko

    2015-03-23

    The Talbot cavity is one promising method to synchronize the phase of a laser array. However, it does not achieve the lowest array mode with the same phase but the highest array mode with the anti-phase between every two adjacent lasers, which is called out-phase locking. Consequently, their far-field images exhibit 2-peak profiles. We propose intra-Talbot-cavity frequency-doubling. By placing a nonlinear crystal in a Talbot cavity, the Talbot cavity generates an out-phased fundamental wave array, which is converted into an in-phase-locked second harmonic wave array at the nonlinear crystal. We demonstrate numerical calculations and experiments on intra-Talbot-cavity frequency-doubling and obtain an in-phase-locked second harmonic wave array for a Nd:YVO₄ array laser.

  14. Second-harmonic generation efficiency for multifrequency ytterbium-doped fibre laser radiation

    SciTech Connect

    Politko, M O; Kablukov, S I; Nemov, I N; Babin, Sergei A

    2013-02-28

    The second-harmonic generation (SHG) efficiency for cw Yb-doped fibre laser radiation, which is characterised by many longitudinal modes with random phases, is compared with the SHG efficiency for amplified single-frequency Nd : YAG laser radiation in ppLN and KTP crystals, characterised by the type-I and type-IIphase matching, respectively. It is shown that the conversion efficiency into the second harmonic in the multifrequency regime for both crystals is higher by a factor of about 1.6, a value close to the calculated enhancement (2 for the Gaussian mode statistics). This difference is explained by possible deviation of the statistics of the Yb-doped fibre laser radiation from Gaussian, which is confirmed by measurements of the laser temporal dynamics. (laser optics 2012)

  15. Simultaneous stimulated Raman scattering and higher harmonic generation imaging for liver disease diagnosis without labeling

    NASA Astrophysics Data System (ADS)

    Lin, Jian; Wang, Zi; Zheng, Wei; Huang, Zhiwei

    2014-02-01

    Nonlinear optical microscopy (e.g., higher harmonic (second-/third- harmonic) generation (HHG), simulated Raman scattering (SRS)) has high diagnostic sensitivity and chemical specificity, making it a promising tool for label-free tissue and cell imaging. In this work, we report a development of a simultaneous SRS and HHG imaging technique for characterization of liver disease in a bile-duct-ligation rat-modal. HHG visualizes collagens formation and reveals the cell morphologic changes associated with liver fibrosis; whereas SRS identifies the distributions of hepatic fat cells formed in steatosis liver tissue. This work shows that the co-registration of SRS and HHG images can be an effective means for label-free diagnosis and characterization of liver steatosis/fibrosis at the cellular and molecular levels.

  16. Harmonization of initial estimates of shale gas life cycle greenhouse gas emissions for electric power generation

    PubMed Central

    Heath, Garvin A.; O’Donoughue, Patrick; Arent, Douglas J.; Bazilian, Morgan

    2014-01-01

    Recent technological advances in the recovery of unconventional natural gas, particularly shale gas, have served to dramatically increase domestic production and reserve estimates for the United States and internationally. This trend has led to lowered prices and increased scrutiny on production practices. Questions have been raised as to how greenhouse gas (GHG) emissions from the life cycle of shale gas production and use compares with that of conventionally produced natural gas or other fuel sources such as coal. Recent literature has come to different conclusions on this point, largely due to differing assumptions, comparison baselines, and system boundaries. Through a meta-analytical procedure we call harmonization, we develop robust, analytically consistent, and updated comparisons of estimates of life cycle GHG emissions for electricity produced from shale gas, conventionally produced natural gas, and coal. On a per-unit electrical output basis, harmonization reveals that median estimates of GHG emissions from shale gas-generated electricity are similar to those for conventional natural gas, with both approximately half that of the central tendency of coal. Sensitivity analysis on the harmonized estimates indicates that assumptions regarding liquids unloading and estimated ultimate recovery (EUR) of wells have the greatest influence on life cycle GHG emissions, whereby shale gas life cycle GHG emissions could approach the range of best-performing coal-fired generation under certain scenarios. Despite clarification of published estimates through harmonization, these initial assessments should be confirmed through methane emissions measurements at components and in the atmosphere and through better characterization of EUR and practices. PMID:25049378

  17. Harmonization of initial estimates of shale gas life cycle greenhouse gas emissions for electric power generation.

    PubMed

    Heath, Garvin A; O'Donoughue, Patrick; Arent, Douglas J; Bazilian, Morgan

    2014-08-01

    Recent technological advances in the recovery of unconventional natural gas, particularly shale gas, have served to dramatically increase domestic production and reserve estimates for the United States and internationally. This trend has led to lowered prices and increased scrutiny on production practices. Questions have been raised as to how greenhouse gas (GHG) emissions from the life cycle of shale gas production and use compares with that of conventionally produced natural gas or other fuel sources such as coal. Recent literature has come to different conclusions on this point, largely due to differing assumptions, comparison baselines, and system boundaries. Through a meta-analytical procedure we call harmonization, we develop robust, analytically consistent, and updated comparisons of estimates of life cycle GHG emissions for electricity produced from shale gas, conventionally produced natural gas, and coal. On a per-unit electrical output basis, harmonization reveals that median estimates of GHG emissions from shale gas-generated electricity are similar to those for conventional natural gas, with both approximately half that of the central tendency of coal. Sensitivity analysis on the harmonized estimates indicates that assumptions regarding liquids unloading and estimated ultimate recovery (EUR) of wells have the greatest influence on life cycle GHG emissions, whereby shale gas life cycle GHG emissions could approach the range of best-performing coal-fired generation under certain scenarios. Despite clarification of published estimates through harmonization, these initial assessments should be confirmed through methane emissions measurements at components and in the atmosphere and through better characterization of EUR and practices. PMID:25049378

  18. Switchable dielectric, piezoelectric, and second-harmonic generation bistability in a new improper ferroelectric above room temperature.

    PubMed

    Zhang, Yi; Ye, Heng-Yun; Cai, Hong-Ling; Fu, Da-Wei; Ye, Qiong; Zhang, Wen; Zhou, Qionghua; Wang, Jinlan; Yuan, Guo-Liang; Xiong, Ren-Gen

    2014-07-01

    Imidazolium periodate (IPI) is found to be an improper ferroelectric. It shows bistable properties simultaneously in three channels of dielectricity, piezoelectricity, and second-harmonic generation within the temperature window 300-310 K. PMID:24789577

  19. Influence of C{sub 60} morphology on high-order harmonic generation enhancement in fullerene-containing plasma

    SciTech Connect

    Ganeev, R. A.; Singhal, H.; Naik, P. A.; Chakera, J. A.; Srivastava, A. K.; Dhami, T. S.; Joshi, M. P.; Gupta, P. D.

    2009-11-15

    The morphologies of the fullerene targets and the ablated fullerenes to determine the optimal conditions of excitation of the C{sub 60}-containing targets have been analyzed. The optimization of fullerene-containing plasma conditions allowed the enhanced harmonic generation in these plasmas using laser radiation of different wavelengths, pulse durations, and phase modulation. A comparison between the harmonic generation in single-atom/ion-containing plasmas (using bulk carbon, silver, and indium targets) and fullerene-rich plasma plumes showed better conversion efficiency for the latter medium. The influence of phase modulation of the fundamental radiation in fullerene plasmas on the spectral properties of harmonics has been studied.

  20. Quasi-phase-matching high harmonic generation using trains of pulses produced using an array of birefringent plates.

    PubMed

    O'Keeffe, Kevin; Robinson, Tom; Hooker, Simon M

    2012-03-12

    Quasi-phase-matched high harmonic generation using trains of up to 8 counter-propagating pulses is explored. For trains of up to 4 pulses the measured enhancement of the harmonic signal scales with the number of pulses N as (N + 1)², as expected. However, for trains with N > 4, no further enhancement of the harmonic signal is observed. This effect is ascribed to changes of the coherence length Lc within the generating medium. Techniques for overcoming the variation of Lc are discussed. The pressure dependence of quasi-phase-matching is investigated and the switch from true-phase-matching to quasi-phase-matching is observed.

  1. A Proof-Of-Principle Echo-Enabled Harmonic Generation Experiment at SLAC

    SciTech Connect

    Dunning, Michael; Colby, Eric; Ding, Yuantao; Frederico, Joel; Gilevich, Sasha; Hast, Carsten; Jobe, R.; McCormick, Douglas; Nelson, Janice; Raubenheimer, Tor; Soong, Ken; Stupakov, Gennady; Szalata, Zenon; Walz, Dieter; Weathersby, Stephen; Woodley, Mark; Xiang, Dao; Corlett, John; Penn, Gregory; Prestemon, Soren; Qiang, Ji; /LBL, Berkeley /LBL, Berkeley /LBL, Berkeley /LBL, Berkeley /LPHE, Lausanne

    2011-05-20

    In this paper we describe the technical design of an ongoing proof-of-principle echo-enabled harmonic generation (EEHG) experiment at the Next Linear Collider Test Accelerator (NLCTA) at SLAC.We present the design considerations and the technical details of the experiment. Recently a new method, entitled echo-enabled harmonic generation, was proposed for generation of high harmonics using the beam echo effect. In an EEHG free electron laser (FEL), an electron beam is energy modulated in a modulator and then sent through a dispersive section with a high dispersion strength. After this first stage, the modulation obtained in the modulator is macroscopically washed out, while simultaneously introducing complicated fine structure (separated energy bands) into the phase space of the beam. A second laser is used to further modulate the beam energy in a second modulator. After passing through a second dispersive section, the separated energy bands will be converted into current modulation and the echo signal then occurs as a recoherence effect caused by the mixing of the correlations between the modulation in the second modulator and the fine structures in the beam. The EEHG scheme has a remarkable up-frequency conversion efficiency; it has been shown that the EEHG FEL scheme may allow generation of soft x-rays directly from a UV seed laser in a single stage. In order to confirm the physics behind the EEHG technique and benchmark the theory, a proof-of-principleEEHG experimentwas planned at SLAC. The experiment is now in a commissioning stage and the preliminary results are reported in a separate paper of these proceedings. In this paper we present the design considerations and the details of the experiment setup.

  2. Single attosecond pulse from terahertz-assisted high-order harmonic generation

    SciTech Connect

    Balogh, Emeric; Kovacs, Katalin; Dombi, Peter; Farkas, Gyozo; Fulop, Jozsef A.; Hebling, Janos; Tosa, Valer; Varju, Katalin

    2011-08-15

    High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the combination of THz fields with up to 12 fs laser pulses can be an effective gating technique to generate single attosecond pulses. We show that in the presence of the strong THz field only a single attosecond burst can be phase matched, whereas radiation emitted during other half cycles disappears during propagation. The cutoff is extended and a wide supercontinuum appears in the near-field spectra, extending the available spectral width for isolated attosecond pulse generation from 23 to 93 eV. We demonstrate that phase-matching effects are responsible for the generation of isolated attosecond pulses, even in conditions when single-atom response yields an attosecond pulse train.

  3. Simulations of high harmonic generation from plasmonic nanoparticles in the terahertz region

    NASA Astrophysics Data System (ADS)

    Grynko, Yevgen; Zentgraf, Thomas; Meier, Torsten; Förstner, Jens

    2016-09-01

    Metallic nanostructures are known for enhancing weak nonlinear processes when a resonant and coherent excitation takes place. With proper structural design, an additional boost of particular nonlinear processes is expected to be possible. Here, we present a numerical technique that is capable of simulating high harmonic generation from resonantly excited metallic nanoparticles in the terahertz frequency range. We demonstrate our method by investigating the nonlinear emission of arrays of plasmonic split-ring resonators at the range of ten terahertzs. Our multiscale, non-perturbative, and microscopic approach is based on a self-consistent combination of a hydrodynamic model for the nonlinear electronic material response and the discontinuous Garlerkin time-domain technique for the evaluation of the propagation of the electromagnetic field. It is predicted that the electronic nonlinearities of plasmonic nanoparticles give rise to several harmonics in the light emission when excited by intense terahertz radiation. Furthermore, our analysis predicts a non-perturbative scaling of higher harmonics at high excitation intensities.

  4. High-harmonic generation by field enhanced femtosecond pulses in metal-sapphire nanostructure

    PubMed Central

    Han, Seunghwoi; Kim, Hyunwoong; Kim, Yong Woo; Kim, Young-Jin; Kim, Seungchul; Park, In-Yong; Kim, Seung-Woo

    2016-01-01

    Plasmonic high-harmonic generation (HHG) drew attention as a means of producing coherent extreme ultraviolet (EUV) radiation by taking advantage of field enhancement occurring in metallic nanostructures. Here a metal-sapphire nanostructure is devised to provide a solid tip as the HHG emitter, replacing commonly used gaseous atoms. The fabricated solid tip is made of monocrystalline sapphire surrounded by a gold thin-film layer, and intended to produce EUV harmonics by the inter- and intra-band oscillations of electrons driven by the incident laser. The metal-sapphire nanostructure enhances the incident laser field by means of surface plasmon polaritons, triggering HHG directly from moderate femtosecond pulses of ∼0.1 TW cm−2 intensities. The measured EUV spectra exhibit odd-order harmonics up to ∼60 nm wavelengths without the plasma atomic lines typically seen when using gaseous atoms as the HHG emitter. This experimental outcome confirms that the plasmonic HHG approach is a promising way to realize coherent EUV sources for nano-scale near-field applications in spectroscopy, microscopy, lithography and atto-second physics. PMID:27721374

  5. Opportunities for chiral discrimination using high harmonic generation in tailored laser fields

    NASA Astrophysics Data System (ADS)

    Smirnova, Olga; Mairesse, Yann; Patchkovskii, Serguei

    2015-12-01

    Chiral discrimination with high harmonic generation (cHHG method) has been introduced in the recent work by R Cireasa et al (2015 Nat. Phys. 11 654-8). In its original implementation, the cHHG method works by detecting high harmonic emission from randomly oriented ensemble of chiral molecules driven by elliptically polarized field, as a function of ellipticity. Here we discuss future perspectives in the development of this novel method, the ways of increasing chiral dichroism using tailored laser pulses, new detection schemes involving high harmonic phase measurements, and concentration-independent approaches. Using the example of the epoxypropane molecule CH3CHCH2O (also known as 1,2-propylene oxide), we show theoretically that application of two-color counter-rotating elliptically polarized laser fields yields an order of magnitude enhancement of chiral dichroism compared to single color elliptical fields. We also describe how one can introduce a new functionality to cHHG: concentration-independent measurement of the enatiomeric excess in a mixture of randomly oriented left-handed and right-handed molecules. Finally, for arbitrary configurations of laser fields, we connect the observables of the cHHG method to the amplitude and phase of chiral response, providing a basis for reconstructing wide range of chiral dynamics from cHHG measurements, with femtosecond to sub-femtosecond temporal resolution.

  6. Characterization of Tissue-Engineered Posterior Corneas Using Second- and Third-Harmonic Generation Microscopy

    PubMed Central

    Jay, Louis; Bourget, Jean-Michel; Goyer, Benjamin; Singh, Kanwarpal; Brunette, Isabelle; Ozaki, Tsuneyuki; Proulx, Stéphanie

    2015-01-01

    Three-dimensional tissues, such as the cornea, are now being engineered as substitutes for the rehabilitation of vision in patients with blinding corneal diseases. Engineering of tissues for translational purposes requires a non-invasive monitoring to control the quality of the resulting biomaterial. Unfortunately, most current methods still imply invasive steps, such as fixation and staining, to clearly observe the tissue-engineered cornea, a transparent tissue with weak natural contrast. Second- and third-harmonic generation imaging are well known to provide high-contrast, high spatial resolution images of such tissues, by taking advantage of the endogenous contrast agents of the tissue itself. In this article, we imaged tissue-engineered corneal substitutes using both harmonic microscopy and classic histopathology techniques. We demonstrate that second- and third-harmonic imaging can non-invasively provide important information regarding the quality and the integrity of these partial-thickness posterior corneal substitutes (observation of collagen network, fibroblasts and endothelial cells). These two nonlinear imaging modalities offer the new opportunity of monitoring the engineered corneas during the entire process of production. PMID:25918849

  7. Visualization of mitochondria in cardiomyocytes by simultaneous harmonic generation and fluorescence microscopy

    NASA Astrophysics Data System (ADS)

    Barzda, Virginijus; Greenhalgh, Catherine; Aus der Au, Jürg; Elmore, Steven; Hgm van Beek, Johannes; Squier, Jeff

    2005-10-01

    The simultaneous detection of third harmonic (THG), and multiphoton excitation fluorescence (MPF) or second harmonic (SHG) from the same focal volume has led us to the development of a nonlinear multimodal microscopic biological imaging tool. The multimodal microscope has been applied for imaging of isolated live cardiomyocytes, and investigation of structural origin of the THG and SHG signals has been performed. By employing the different image contrast mechanisms, differentiation of structures inside a single live adult rat cardiomyocyte has been achieved. Based on structural crosscorrelation image analysis between NAD(P)H fluorescence and THG, and morphology of cardiomyocytes we were able to assign large part of the structure revealed by THG to the mitochondria. The crosscorrelation of THG with fluorescence of tetramethylrhodamine methyl ester (TMRM) labeled cardiomyocytes confirmed the mitochondrial origin of THG. The SHG generated structures were anticorrelated with THG and possessed the characteristic pattern of the myofibrils in the myocyte in accordance with the literature. Possible visualization of mitochondria with THG microscopy appeared due to enhancement of the third harmonic by multilayer arrangement of cristae.

  8. High-harmonic generation by field enhanced femtosecond pulses in metal-sapphire nanostructure

    NASA Astrophysics Data System (ADS)

    Han, Seunghwoi; Kim, Hyunwoong; Kim, Yong Woo; Kim, Young-Jin; Kim, Seungchul; Park, In-Yong; Kim, Seung-Woo

    2016-10-01

    Plasmonic high-harmonic generation (HHG) drew attention as a means of producing coherent extreme ultraviolet (EUV) radiation by taking advantage of field enhancement occurring in metallic nanostructures. Here a metal-sapphire nanostructure is devised to provide a solid tip as the HHG emitter, replacing commonly used gaseous atoms. The fabricated solid tip is made of monocrystalline sapphire surrounded by a gold thin-film layer, and intended to produce EUV harmonics by the inter- and intra-band oscillations of electrons driven by the incident laser. The metal-sapphire nanostructure enhances the incident laser field by means of surface plasmon polaritons, triggering HHG directly from moderate femtosecond pulses of ~0.1 TW cm-2 intensities. The measured EUV spectra exhibit odd-order harmonics up to ~60 nm wavelengths without the plasma atomic lines typically seen when using gaseous atoms as the HHG emitter. This experimental outcome confirms that the plasmonic HHG approach is a promising way to realize coherent EUV sources for nano-scale near-field applications in spectroscopy, microscopy, lithography and atto-second physics.

  9. Size dependence of second-harmonic generation at the surface of microspheres

    NASA Astrophysics Data System (ADS)

    Viarbitskaya, Sviatlana; Kapshai, Valery; van der Meulen, Peter; Hansson, Tony

    2010-05-01

    The resonance-enhanced surface second-harmonic generation (SHG) from a suspension of polystyrene microspheres was investigated as a function of particle size in a range of the order of the fundamental wavelength for two different second-harmonic-enhancing dyes—malachite green and pyridine 1. The two dyes gave the same strongly modulated pattern of the forward second-harmonic scattering efficiency. Direct comparison to the nonlinear Rayleigh-Gans-Debye (NLRGD) and nonlinear Wentzel-Kramers-Brillouin (NLWKB) model predictions showed that the NLWKB model reproduces the overall trend in the size dependence but fails with respect to the strong modulations. The standard NLRGD model was found to fail altogether in the present particle size range, which was well beyond the observed upper particle size for which the NLRGD and NLWKB models give comparable results. A generalization of the NLRGD model to allow for dispersion and to use the particle refractive indices instead of those of the surrounding medium extended its applicability range by almost an order of magnitude in particle size. There is a pronounced maximal SHG efficiency for particles with a radius that is close to the fundamental wavelength inside the particle. The optically soft particle approximation is inadequate to describe the SHG in this particle size range, as refraction and reflection of the waves at the particle surface have a decisive influence. Dispersion of the media plays a negligible role for particle sizes up to about twice the optimal one for SHG.

  10. Size dependence of second-harmonic generation at the surface of microspheres

    SciTech Connect

    Viarbitskaya, Sviatlana; Meulen, Peter van der; Hansson, Tony; Kapshai, Valery

    2010-05-15

    The resonance-enhanced surface second-harmonic generation (SHG) from a suspension of polystyrene microspheres was investigated as a function of particle size in a range of the order of the fundamental wavelength for two different second-harmonic-enhancing dyes--malachite green and pyridine 1. The two dyes gave the same strongly modulated pattern of the forward second-harmonic scattering efficiency. Direct comparison to the nonlinear Rayleigh-Gans-Debye (NLRGD) and nonlinear Wentzel-Kramers-Brillouin (NLWKB) model predictions showed that the NLWKB model reproduces the overall trend in the size dependence but fails with respect to the strong modulations. The standard NLRGD model was found to fail altogether in the present particle size range, which was well beyond the observed upper particle size for which the NLRGD and NLWKB models give comparable results. A generalization of the NLRGD model to allow for dispersion and to use the particle refractive indices instead of those of the surrounding medium extended its applicability range by almost an order of magnitude in particle size. There is a pronounced maximal SHG efficiency for particles with a radius that is close to the fundamental wavelength inside the particle. The optically soft particle approximation is inadequate to describe the SHG in this particle size range, as refraction and reflection of the waves at the particle surface have a decisive influence. Dispersion of the media plays a negligible role for particle sizes up to about twice the optimal one for SHG.

  11. Role of quantum trajectory in high-order harmonic generation in the Keldysh multiphoton regime

    NASA Astrophysics Data System (ADS)

    Li, Peng-Cheng; Chu, Shih-I.

    2016-05-01

    We present a systematic study of quantum-trajectory analysis of high-order harmonic generation (HHG) by solving accurately the time-dependent Schrödinger equation for a hydrogen atom in the multiphoton regime where the Keldysh parameter is greater unity. We perform the time-frequency transform to explore the spectral characteristics of the HHG. We find that the time-frequency spectra exhibit a broken distribution at above-threshold HHG due to the competition associated with the short- and long-trajectories when the ionization process is pushed from the multiphoton regime into the tunneling regime, it implies that the harmonic emission in the broken regions of time-frequency spectra are suppressed. In addition, we present a time-dependent density-functional theory approach for an ab initio study of the effect of correlated multielectron responses on the harmonic emission of Ar atom associated with the quantum trajectories in the multiphoton regime. This work is partially supported by DOE.

  12. Long-term operation of surface high-harmonic generation from relativistic oscillating mirrors using a spooling tape

    SciTech Connect

    Bierbach, Jana; Yeung, Mark; Eckner, Erich; Roedel, Christian; Kuschel, Stephan; Zepf, Matt; Paulus, Gerhard G.

    2015-05-01

    Surface high-harmonic generation in the relativistic regime is demonstrated as a source of extreme ultra-violet (XUV) pulses with extended operation time. Relativistic high-harmonic generation is driven by a frequency-doubled high-power Ti:Sapphire laser focused to a peak intensity of 3·1019 W/cm2 onto spooling tapes. We demonstrate continuous operation over up to one hour runtime at a repetition rate of 1 Hz. Harmonic spectra ranging from 20 eV to 70 eV (62 nm to 18 nm) were consecutively recorded by an XUV spectrometer. An average XUV pulse energy in the µJ range is measured. With the presented setup, relativistic surface high-harmonic generation becomes a powerful source of coherent XUV pulses that might enable applications in, e.g. attosecond laser physics and the seeding of free-electron lasers, when the laser issues causing 80-% pulse energy fluctuations are overcome.

  13. Single-pass high harmonic generation at high repetition rate and photon flux

    NASA Astrophysics Data System (ADS)

    Hädrich, Steffen; Rothhardt, Jan; Krebs, Manuel; Demmler, Stefan; Klenke, Arno; Tünnermann, Andreas; Limpert, Jens

    2016-09-01

    Sources of short wavelength radiation with femtosecond to attosecond pulse durations, such as synchrotrons or free electron lasers, have already made possible numerous, and will facilitate more, seminal studies aimed at understanding atomic and molecular processes on fundamental length and time scales. Table-top sources of coherent extreme ultraviolet to soft x-ray radiation enabled by high harmonic generation (HHG) of ultrashort pulse lasers have also gained significant attention in the last few years due to their enormous potential for addressing a plethora of applications, therefore constituting a complementary source to large-scale facilities (synchrotrons and free electron lasers). Ti:sapphire based laser systems have been the workhorses for HHG for decades, but are limited in repetition rate and average power. On the other hand, it has been widely recognized that fostering applications in fields such as photoelectron spectroscopy and microscopy, coincidence detection, coherent diffractive imaging and frequency metrology requires a high repetition rate and high photon flux HHG sources. In this article we will review recent developments in realizing the demanding requirement of producing a high photon flux and repetition rate at the same time. Particular emphasis will be put on suitable ultrashort pulse and high average power lasers, which directly drive harmonic generation without the need for external enhancement cavities. To this end we describe two complementary schemes that have been successfully employed for high power fiber lasers, i.e. optical parametric chirped pulse amplifiers and nonlinear pulse compression. Moreover, the issue of phase-matching in tight focusing geometries will be discussed and connected to recent experiments. We will highlight the latest results in fiber laser driven high harmonic generation that currently produce the highest photon flux of all existing sources. In addition, we demonstrate the first promising applications and

  14. Laser absorption and third-harmonic generation in free-electron nanofilms

    SciTech Connect

    Fomichev, Sergey V.; Zaretsky, David F.; Becker, Wilhelm

    2009-02-15

    The collective collisionless dynamics of the electron gas in free-electron nanofilms irradiated by an obliquely incident p-polarized laser wave are considered in the classical hydrodynamic and jellium-model approximations. The two cases of cold metallic nanofilms and hot free-electron nanofilms laser ionized and laser heated by a pump-laser prepulse are investigated with proper electron statistics. Both linear and nonlinear properties of the plasma resonance excitation in the nanofilms are studied in detail for different film parameters (film thickness, thickness of the diffuse film boundary, outer-ionization degree for hot laser-ionized/heated films, etc.). The significant role of the diffuse film boundaries for both linear absorption of the laser field and third-harmonic generation is demonstrated. For this goal, we do not use the standard dielectric-permittivity approach with boundary conditions between two different media but solve continuously over all space the full set of hydrodynamic and electrodynamic equations in nonrelativistic one-dimensional approximation. It is shown that collisionless edge absorption may be dominant in thin nanofilms, while in cold metal nanofilms it results in the appearance of several linear-absorption resonances below the bulk-plasma resonance frequency. For hot nanofilms, drastic broadening of the linear-plasma-resonance profile is obtained in calculations when the film thickness is reduced. In our model, the third-harmonic generation is determined by the density gradient in the diffuse film edges. Additional resonances in third-harmonic generation as a function of laser frequency are obtained for cold metal nanofilms. They differ from the standard third-order nonlinear resonance, which is located at one third of the plasma resonance frequency. The important role of the outer-ionization degree in forming the third-order nonlinear response of the hot laser-ionized film is also analyzed and discussed.

  15. Third-harmonic generation microscopy reveals dental anatomy in ancient fossils.

    PubMed

    Chen, Yu-Cheng; Lee, Szu-Yu; Wu, Yana; Brink, Kirstin; Shieh, Dar-Bin; Huang, Timothy D; Reisz, Robert R; Sun, Chi-Kuang

    2015-04-01

    Fossil teeth are primary tools in the study of vertebrate evolution, but standard imaging modalities have not been capable of providing high-quality images in dentin, the main component of teeth, owing to small refractive index differences in the fossilized dentin. Our first attempt to use third-harmonic generation (THG) microscopy in fossil teeth has yielded significant submicrometer level anatomy, with an unexpectedly strong signal contrasting fossilized tubules from the surrounding dentin. Comparison between fossilized and extant teeth of crocodilians reveals a consistent evolutionary signature through time, indicating the great significance of THG microscopy in the evolutionary studies of dental anatomy in fossil teeth.

  16. Cell tracking in live Caenorhabditis elegans embryos via third harmonic generation imaging microscopy measurements

    NASA Astrophysics Data System (ADS)

    Tserevelakis, George J.; Filippidis, George; Megalou, Evgenia V.; Fotakis, Costas; Tavernarakis, Nektarios

    2011-04-01

    In this study, we demonstrate the potential of employing third harmonic generation (THG) imaging microscopy measurements for cell tracking studies in live Caenorhabditis elegans (C. elegans) embryos. A 1028-nm femtosecond laser was used for the excitation of unstained C. elegans samples. Different C. elegans embryonic stages (from two-cell to threefold) were imaged. Live biological specimens were irradiated for prolonged periods of time (up to 7 h), testifying to the nondestructive nature of this nonlinear imaging technique. Thus, THG image contrast modality is a powerful diagnostic tool for probing in vivo cell division during early embryogenesis.

  17. Velocimetric third-harmonic generation microscopy: micrometer-scale quantification of morphogenetic movements in unstained embryos

    NASA Astrophysics Data System (ADS)

    Débarre, Delphine; Supatto, Willy; Farge, Emmanuel; Moulia, Bruno; Schanne-Klein, Marie-Claire; Beaurepaire, Emmanuel

    2004-12-01

    We demonstrate the association of third-harmonic generation (THG) microscopy and particle image velocimetry (PIV) analysis as a novel functional imaging technique for automated micrometer-scale characterization of morphogenetic movements in developing embryos. Using a combined two-photon-excited fluorescence and THG microscope, we characterize the optical properties of Drosophila embryos and show that sustained THG imaging does not perturb sensitive developmental dynamics. Velocimetric THG imaging provides a quantitative description of the dynamics of internal structures in unstained wild-type and mutant embryos.

  18. Ultrastructural features of collagen in thyroid carcinoma tissue observed by polarization second harmonic generation microscopy

    PubMed Central

    Tokarz, Danielle; Cisek, Richard; Golaraei, Ahmad; Asa, Sylvia L.; Barzda, Virginijus; Wilson, Brian C.

    2015-01-01

    Changes in collagen ultrastructure between malignant and normal human thyroid tissue were investigated ex vivo using polarization second harmonic generation (SHG) microscopy. The second-order nonlinear optical susceptibility tensor component ratio and the degree of linear polarization (DOLP) of the SHG signal were measured. The ratio values are related to the collagen ultrastructure, while DOLP indicates the relative amount of coherent signal and incoherent scattering of SHG. Increase in ratio values and decrease in DOLP were observed for tumor tissue compared to normal thyroid, indicating higher ultrastructural disorder in tumor collagen. PMID:26417516

  19. Frequency dependence of optical third-harmonic generation from doped graphene

    NASA Astrophysics Data System (ADS)

    Margulis, Vl. A.; Muryumin, E. E.; Gaiduk, E. A.

    2016-01-01

    In connection with the controversial question about the frequency dependence of the optical third-harmonic generation (THG) from doped graphene, which has recently been discussed in the literature, we develop an analytical theory for the THG susceptibility of doped graphene by using the original Genkin-Mednis nonlinear-conductivity-theory formalism including mixed intra- and interband terms. The theory is free of any nonphysical divergences at zero frequency, and it predicts the main resonant peak in the THG spectrum to be located at the photon energy ħω equal to two thirds of the Fermi energy EF of charge carriers in doped graphene.

  20. Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films

    SciTech Connect

    Luk, Ting S. Liu, Sheng; Campione, Salvatore; Ceglia, Domenico de; Vincenti, Maria A.; Keeler, Gordon A.; Sinclair, Michael B.; Prasankumar, Rohit P.; Scalora, Michael

    2015-04-13

    We experimentally demonstrate efficient third harmonic generation from an indium tin oxide nanofilm (λ/42 thick) on a glass substrate for a pump wavelength of 1.4 μm. A conversion efficiency of 3.3 × 10{sup −6} is achieved by exploiting the field enhancement properties of the epsilon-near-zero mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.

  1. Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films

    SciTech Connect

    Luk, Ting S.; De Ceglia, Domenico; Liu, Sheng; Keeler, Gordon Arthur; Prasankumar, Rohit; Los Alamos National Lab. , Los Alamos, NM ; Vincenti, Maria A; Scalora, Michael; Sinclair, Michael B.; campione, salvatore

    2015-04-13

    We demonstrate, through our experimentation, efficient third harmonic generation from an indium tin oxide nanofilm (λ/42 thick) on a glass substrate for a pump wavelength of 1.4 μm. A conversion efficiency of 3.3 × 10-6 is achieved by exploiting the field enhancement properties of the epsilon-near-zero mode with an enhancement factor of 200. Furthermore, this nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.

  2. Broadband second harmonic generation in an imperfect nonlinear photonic crystal with random defects

    NASA Astrophysics Data System (ADS)

    Ren, Kun; Liu, Yali; Ren, Xiaobin; Fan, Jingyang

    2016-09-01

    In this paper, we study broadband second harmonic generation (SHG) in an imperfect nonlinear photonic crystal in which defects are introduced with random lengths. We show that the efficient SHG output is obtained when the length of each defect varies near certain specialized values. The bandwidth of the SHG output broadens with the increasing randomness of defect length. Moreover, the SHG bandwidth is nearly unaffected only when the total length of the whole structure is long enough. The disordered structure also exhibits good tolerance to the fabrication error, which provides a way to control SHG intensity and bandwidth separately.

  3. Perturbation theory for graphene-integrated waveguides: Cubic nonlinearity and third-harmonic generation

    NASA Astrophysics Data System (ADS)

    Gorbach, Andrey V.; Ivanov, Edouard

    2016-07-01

    We present perturbation theory for analysis of generic third-order nonlinear processes in graphene-integrated photonic structures. The optical response of graphene is treated as the nonlinear boundary condition in Maxwell's equations. The derived models are applied for analysis of third-harmonic generation in a graphene-coated dielectric microfiber. An efficiency of up to a few percent is predicted when using subpicosecond pump pulses with energies of the order of 0.1 nJ in a submillimeter-long fiber when operating near the resonance of the graphene nonlinear conductivity ℏ ω =(2 /3 ) EF .

  4. Study of the second harmonic generation and optical rectification in a cBN crystal

    SciTech Connect

    Dou Qingping; Ma Haitao; Jia Gang; Chen Zhanguo; Cao Kun; Zhang Tiechen

    2007-02-28

    Cubic boron nitride (cBN) - a kind of an artificial (synthetic) crystal with the band gap of {approx}6.3 eV, which has the zinc blende structure and the 4-bar 3m symmetry, is studied. The optical rectification is obtained and the second harmonic generation (SHG) is observed in the cBN crystal for the first time by using a 1064-nm Q-switched Nd:YAG laser. The green light at 532 nm from the cBN sample can be seen with a naked eye. (nonlinear optical phenomena)

  5. Discrimination of collagen in normal and pathological dermis through polarization second harmonic generation

    NASA Astrophysics Data System (ADS)

    Su, Ping-Jung; Chen, Wei-Liang; Hong, Jin-Bon; Li, Tsung-Hsien; Wu, Ruei-Jr; Chou, Chen-Kuan; Lin, Sung-Jan; Dong, Chen-Yuan

    2010-02-01

    We used polarization-resolved, second harmonic generation (P-SHG) microscopy at single pixel resolution for medical diagnosis of pathological skin dermis, and found that P-SHG can be used to distinguish normal and dermal pathological conditions of keloid, morphea, and dermal elastolysis. We find that the histograms of the d33/d31 ratio for the pathological skins to contain two peak values and to be wider than that of the normal case, suggesting that the pathological dermal collagen fibers tend to be more structurally heterogeneous. Our work demonstrates that pixel-resolved, second-order susceptibility microscopy is effective for detecting heterogeneity in spatial distribution of collagen fibers.

  6. Quantitative biomarkers of human skin photoaging based on intrinsic second harmonic generation signal.

    PubMed

    Zhuo, Shuangmu; Zhu, Xiaoqin; Chen, Jianxin; Xie, Shusen

    2013-01-01

    Collagen change is a major feature in the photoaged human skin. Here, we present the use of intrinsic second harmonic generation (SHG) signal as a novel means to quantify collagen change with photoaging. We obtain the SHG images of the superficial dermis from ex vivo the cheek skin and the abdomen skin of eight patients aged 55-60 years. The results show that SHG signal can quantitatively reveal collagen change between normal and photoaged human skin in three dimensions. By comparing normal with photoaged dermis, there are significant differences in the collagen content and fine structure, providing substantial potential to be applied in vivo for the clinical diagnosis of human skin photoaging.

  7. Quantitative biomarkers of colonic dysplasia based on intrinsic second-harmonic generation signal.

    PubMed

    Zhuo, Shuangmu; Zhu, Xiaoqin; Wu, Guizhu; Chen, Jianxin; Xie, Shusen

    2011-12-01

    Most colorectal cancers arise from dysplastic lesions, such as adenomatous polyps, and these lesions are difficult to be detected by the current endoscopic screening approaches. Here, we present the use of an intrinsic second-harmonic generation (SHG) signal as a novel means to differentiate between normal and dysplastic human colonic tissues. We find that the SHG signal can quantitatively identify collagen change associated with colonic dysplasia that is indiscernible by conventional pathologic techniques. By comparing normal with dysplastic mucosa, there were significant differences in collagen density and collagen fiber direction, providing substantial potential to become quantitative intrinsic biomarkers for in vivo clinical diagnosis of colonic dysplasia.

  8. Impact of longitudinal fields on second harmonic generation in lithium niobate nanopillars

    NASA Astrophysics Data System (ADS)

    Baghban, Mohammad Amin; Gallo, Katia

    2016-09-01

    An optimized focused ion beam process is used to fabricate micrometer-long LiNbO3 nanopillars with diameters varying between 150 and 325 nm. Polarimetric mappings of second harmonic generation from a wavelength of 850 nm demonstrate the ability to modify the polarization features of the nonlinear response through a fine adjustment of the pillar size. The effect is ascribed to the non-negligible contribution of the longitudinal fields associated with sub-wavelength light confinement in the LiNbO3 nanopillars. The results also highlight the importance of a fine control over the nanopillar size in order to effectively engineer their nonlinear response.

  9. Electric field-induced second harmonic generation studies of chromophore orientational dynamics in photorefractive polymers

    NASA Astrophysics Data System (ADS)

    Ostroverkhova, Oksana; Stickrath, Andrew; Singer, Kenneth D.

    2002-06-01

    Photorefractive (PR) polymers are promising for use in various applications that require fast response times. The main factors that determine the PR speed in polymers are photoconductivity and chromophore reorientation in an electric field. In this article, we investigate the chromophore reorientational dynamics in various PR composites using the electric field second harmonic generation (EFISHG) technique, and then relate it to the PR dynamics observed in a four-wave mixing holographic experiment. We also report on the enhancement of the EFISHG signal in the presence of HeNe light, which we attribute to a photoinduced internal electric field that formed in the PR polymer.

  10. Nanoscale optical properties of metal nanoparticles probed by Second Harmonic Generation microscopy.

    PubMed

    Shen, Hong; Nguyen, Ngoc; Gachet, David; Maillard, Vincent; Toury, Timothée; Brasselet, Sophie

    2013-05-20

    We report spatial and vectorial imaging of local fields' confinement properties in metal nanoparticles with branched shapes, using Second Harmonic Generation (SHG) microscopy. Taking advantage of the coherent nature of this nonlinear process, the technique provides a direct evidence of the coupling between the excitation polarization and both localization and polarization specificities of local fields at the sub-diffraction scale. These combined features, which are governed by the nanoparticles' symmetry, are not accessible using other contrasts such as linear optical techniques or two-photon luminescence.

  11. Universality of returning electron wave packet in high-order harmonic generation with midinfrared laser pulses.

    PubMed

    Le, Anh-Thu; Wei, Hui; Jin, Cheng; Tuoc, Vu Ngoc; Morishita, Toru; Lin, C D

    2014-07-18

    We show that a returning electron wave packet in high-order harmonic generation (HHG) with midinfrared laser pulses converges to a universal limit for a laser wavelength above about 3 μm. The results are consistent among the different methods: a numerical solution of the time-dependent Schrödinger equation, the strong-field approximation, and the quantum orbits theory. We further analyze how the contribution from different electron "trajectories" survives the macroscopic propagation in the medium. Our result thus provides a new framework for investigating the wavelength scaling law for the HHG yields.

  12. Improved and enhanced thermal stable second harmonic generation of poled polymer films

    NASA Astrophysics Data System (ADS)

    Hou, Zhanjia; Liu, Liying; Liu, Haibo; Xu, Lei; Wang, Wencheng; Li, Fuming; Ye, Mingxin

    2000-11-01

    Melamine formaldehyde resin films with good optical quality could be fabricated easily by controlling the initial molecular weight. It was used as a matrix of nonlinear molecules. The optical properties of nonlinear molecules guest-host and covalent-bonded type of poled polymer systems were investigated. The optical propagation losses are around 1 dB/cm at 1072 nm for two kinds of films studied. The in situ corona poling second harmonic generation method and UV- visible absorption measurement were used. The experiment results showed that the materials we fabricated have improved second-order susceptibilities and higher thermal stability.

  13. Label-free three-dimensional imaging of cell nucleus using third-harmonic generation microscopy

    NASA Astrophysics Data System (ADS)

    Lin, Jian; Zheng, Wei; Wang, Zi; Huang, Zhiwei

    2014-09-01

    We report the implementation of the combined third-harmonic generation (THG) and two-photon excited fluorescence (TPEF) microscopy for label-free three-dimensional (3-D) imaging of cell nucleus morphological changes in liver tissue. THG imaging shows regular spherical shapes of normal hepatocytes nuclei with inner chromatin structures while revealing the condensation of chromatins and nuclear fragmentations in hepatocytes of diseased liver tissue. Colocalized THG and TPEF imaging provides complementary information of cell nuclei and cytoplasm in tissue. This work suggests that 3-D THG microscopy has the potential for quantitative analysis of nuclear morphology in cells at a submicron-resolution without the need for DNA staining.

  14. Label-free three-dimensional imaging of cell nucleus using third-harmonic generation microscopy

    SciTech Connect

    Lin, Jian; Zheng, Wei; Wang, Zi; Huang, Zhiwei

    2014-09-08

    We report the implementation of the combined third-harmonic generation (THG) and two-photon excited fluorescence (TPEF) microscopy for label-free three-dimensional (3-D) imaging of cell nucleus morphological changes in liver tissue. THG imaging shows regular spherical shapes of normal hepatocytes nuclei with inner chromatin structures while revealing the condensation of chromatins and nuclear fragmentations in hepatocytes of diseased liver tissue. Colocalized THG and TPEF imaging provides complementary information of cell nuclei and cytoplasm in tissue. This work suggests that 3-D THG microscopy has the potential for quantitative analysis of nuclear morphology in cells at a submicron-resolution without the need for DNA staining.

  15. Materials characterization using acoustic nonlinearity parameters and harmonic generation - Engineering materials

    NASA Technical Reports Server (NTRS)

    Yost, William T.; Cantrell, John H.

    1990-01-01

    The paper reviews nonlinear bulk compressional wave acoustic measurement systems and the applications of measurements from such systems to engineering materials. Preliminary measurements indicate that it is possible to determine percent second phase precipitates in aluminum alloys, while other measurements show promise in the determination of properties related to the fatigue states of metals. It is also shown that harmonic generation can be used for the study of crack opening loads in compact tension specimens, which in turn gives useful information about the fatigue properties of various engineering materials.

  16. Fringe-free, Background-free, Collinear Third Harmonic Generation FROG Measurements for Multiphoton Microscopy

    SciTech Connect

    Chadwick, R; Spahr, E; Squier, J A; Durfee, C G; Walker, B C; Fittinghoff, D N

    2006-07-21

    Collinear pulse measurement tools useful at the full numerical aperture (NA) of multiphoton microscope objectives are a necessity for a quantitative characterization of the femtosecond pulses focused by these systems. In this letter, we demonstrate a simple new technique, for characterizing the pulse at the focus in a multiphoton microscope. This technique, a background-free, fringe-free, form of frequency-resolved optical gating, uses the third harmonic signal generated from a glass coverslip. Here it is used to characterize 100 fs pulses (typical values for a multiphoton microscope) at the focus of a 0.65 NA objective.

  17. Multiphoton excited hemoglobin fluorescence and third harmonic generation for non-invasive microscopy of stored blood

    PubMed Central

    Saytashev, Ilyas; Glenn, Rachel; Murashova, Gabrielle A.; Osseiran, Sam; Spence, Dana; Evans, Conor L.; Dantus, Marcos

    2016-01-01

    Red blood cells (RBC) in two-photon excited fluorescence (TPEF) microscopy usually appear as dark disks because of their low fluorescent signal. Here we use 15fs 800nm pulses for TPEF, 45fs 1060nm pulses for three-photon excited fluorescence, and third harmonic generation (THG) imaging. We find sufficient fluorescent signal that we attribute to hemoglobin fluorescence after comparing time and wavelength resolved spectra of other expected RBC endogenous fluorophores: NADH, FAD, biliverdin, and bilirubin. We find that both TPEF and THG microscopy can be used to examine erythrocyte morphology non-invasively without breaching a blood storage bag. PMID:27699111

  18. Magnetic field measurements of a superconducting undulator for a Harmonic Generation FEL experiment at the NSLS

    SciTech Connect

    Solomon, L.; Ingold, G.; Ben-Zvi, I.; Krinsky, S.; Yu, L.H.; Sampson, W.; Robins, K.

    1993-07-01

    An 18mm period, 0.54 Tesla, 8mm gap superconducting undulator with both horizontal and vertical focusing has been built and tested. This magnet, which is fabricated in 25 cm length sections, is being tested for use in the radiator section (total magnet length of 1.5 m) of the Harmonic Generation Free Electron Laser experiment at the National Synchrotron Light Source - Accelerator Test Facility at Brookhaven National Lab., in collaboration with Grumman Corp. The measurement system is outlined, sources and estimates of errors are described, and some magnetic field data are presented and discussed.

  19. Molecular Adsorption on Nano Colloidal Particles Probed by Second Harmonic Generation

    NASA Astrophysics Data System (ADS)

    Jen, Shih-Hui; Dai, Hai-Lung

    2006-03-01

    It is shown that second-harmonic generation (SHG), detected at 90 degree angle from the fundamental beam propagation direction, can be used to probe molecular adsorption on spherical nano colloidal particles with diameter as small as 50 nm. Measurements done with the malachite green dye adsorbed on polystyrene particles with diameters ranging from 50 to 250 nm show that the SHG signal from these surface adsorbed molecules tilts toward larger scattering angles when the particle size becomes smaller. This phenomenon can be rigorously described by the nonlinear Rayleigh-Gans-Debye theory and used for measuring the density and adsorption free energy of molecules adsorbed on nanometer size colloidal particles.

  20. Enhanced third harmonic generation in a silicon metasurface using trapped mode.

    PubMed

    Tong, Wenyuan; Gong, Cheng; Liu, Xiaojun; Yuan, Shuai; Huang, Qingzhong; Xia, Jinsong; Wang, Yi

    2016-08-22

    We experimentally demonstrate enhanced third harmonic generation (THG) using a silicon metasurface, which is consist of symmetric spindle-shape nanoparticle array. Relying on the trapped mode supported by the high quality factor all-dielectric metasurface, the conversion efficiency of THG is about 300 times larger than that of bulk silicon slab. The maximum extinction ratio of the intensity of THG reaches about 25 dB by tuning the polarization of incident light. The simulation results agree with the experimental performances. PMID:27557244

  1. Resolution and contrast enhancement of subtractive second harmonic generation microscopy with a circularly polarized vortex beam

    PubMed Central

    Tian, Nian; Fu, Ling; Gu, Min

    2015-01-01

    We extend the subtractive imaging method to label-free second harmonic generation (SHG) microscopy to enhance the spatial resolution and contrast. This method is based on the intensity difference between two images obtained with circularly polarized Gaussian and doughnut-shaped beams, respectively. By characterizing the intensity and polarization distributions of the two focused beams, we verify the feasibility of the subtractive imaging method in polarization dependent SHG microscopy. The resolution and contrast enhancement in different biological samples is demonstrated. This work will open a new avenue for the applications of SHG microscopy in biomedical research. PMID:26364733

  2. Multiphoton excited hemoglobin fluorescence and third harmonic generation for non-invasive microscopy of stored blood

    PubMed Central

    Saytashev, Ilyas; Glenn, Rachel; Murashova, Gabrielle A.; Osseiran, Sam; Spence, Dana; Evans, Conor L.; Dantus, Marcos

    2016-01-01

    Red blood cells (RBC) in two-photon excited fluorescence (TPEF) microscopy usually appear as dark disks because of their low fluorescent signal. Here we use 15fs 800nm pulses for TPEF, 45fs 1060nm pulses for three-photon excited fluorescence, and third harmonic generation (THG) imaging. We find sufficient fluorescent signal that we attribute to hemoglobin fluorescence after comparing time and wavelength resolved spectra of other expected RBC endogenous fluorophores: NADH, FAD, biliverdin, and bilirubin. We find that both TPEF and THG microscopy can be used to examine erythrocyte morphology non-invasively without breaching a blood storage bag.

  3. Simultaneous stimulated Raman scattering and second harmonic generation in periodically poled lithium niobate

    NASA Astrophysics Data System (ADS)

    McConnell, Gail; Ferguson, Allister I.

    2005-03-01

    Simultaneous stimulated Raman scattering (SRS) and second harmonic generation (SHG) are demonstrated in periodically poled lithium niobate (PPLN). Using a simple single-pass geometry, conversion efficiencies of up to 12% and 19% were observed for the SRS and SHG processes respectively. By changing the PPLN period interacting with the photonic crystal fibre based pump source and varying the PPLN temperature, the SHG signal was measured to be tunable from λ =584 nm to λ =679 nm. The SRS output spectrum was measured at λ=1583 nm, with a spectral full-width at half-maximum of λ =85 nm.

  4. Second harmonic generation imaging of collagen fibrils in cornea and sclera

    NASA Astrophysics Data System (ADS)

    Han, Meng; Giese, Günter; Bille, Josef F.

    2005-07-01

    Collagen, as the most abundant protein in the human body, determines the unique physiological and optical properties of the connective tissues including cornea and sclera. The ultrastructure of collagen, which conventionally can only be resolved by electron microscopy, now can be probed by optical second harmonic generation (SHG) imaging. SHG imaging revealed that corneal collagen fibrils are regularly packed as a polycrystalline lattice, accounting for the transparency of cornea. In contrast, scleral fibrils possess inhomogeneous, tubelike structures with thin hard shells, maintaining the high stiffness and elasticity of the sclera.

  5. Ab initio description of second-harmonic generation from crystal surfaces

    NASA Astrophysics Data System (ADS)

    Tancogne-Dejean, Nicolas; Giorgetti, Christine; Véniard, Valérie

    2016-09-01

    We propose an ab initio framework to derive the dielectric and the second-order susceptibility tensors for crystal surfaces. The single-surface response is extracted from a supercell scheme. We evaluate macroscopic quantities, taking into account the local fields. The first- and second-order susceptibilities are evaluated within time-dependent density functional theory, in the long-wavelength limit. We apply our formalism to the calculation of the second-harmonic generation for clean and hydrogenated silicon surfaces. The agreement with measured second-order susceptibility components is significantly better, illustrating the importance of local-field effects.

  6. Third harmonic generation imaging for fast, label-free pathology of human brain tumors.

    PubMed

    Kuzmin, N V; Wesseling, P; Hamer, P C de Witt; Noske, D P; Galgano, G D; Mansvelder, H D; Baayen, J C; Groot, M L

    2016-05-01

    In brain tumor surgery, recognition of tumor boundaries is key. However, intraoperative assessment of tumor boundaries by the neurosurgeon is difficult. Therefore, there is an urgent need for tools that provide the neurosurgeon with pathological information during the operation. We show that third harmonic generation (THG) microscopy provides label-free, real-time images of histopathological quality; increased cellularity, nuclear pleomorphism, and rarefaction of neuropil in fresh, unstained human brain tissue could be clearly recognized. We further demonstrate THG images taken with a GRIN objective, as a step toward in situ THG microendoscopy of tumor boundaries. THG imaging is thus a promising tool for optical biopsies.

  7. Third-harmonic generation microscopy reveals dental anatomy in ancient fossils.

    PubMed

    Chen, Yu-Cheng; Lee, Szu-Yu; Wu, Yana; Brink, Kirstin; Shieh, Dar-Bin; Huang, Timothy D; Reisz, Robert R; Sun, Chi-Kuang

    2015-04-01

    Fossil teeth are primary tools in the study of vertebrate evolution, but standard imaging modalities have not been capable of providing high-quality images in dentin, the main component of teeth, owing to small refractive index differences in the fossilized dentin. Our first attempt to use third-harmonic generation (THG) microscopy in fossil teeth has yielded significant submicrometer level anatomy, with an unexpectedly strong signal contrasting fossilized tubules from the surrounding dentin. Comparison between fossilized and extant teeth of crocodilians reveals a consistent evolutionary signature through time, indicating the great significance of THG microscopy in the evolutionary studies of dental anatomy in fossil teeth. PMID:25831331

  8. Atmospheric thermometry for metallic surfaces by laser-induced second-harmonic generation

    NASA Astrophysics Data System (ADS)

    Pedanekar, Niranjan R.; Yin, Huiqi; Laurendeau, Normand M.

    1996-07-01

    To the best of our knowledge we report the first demonstration of surface thermometry using laser-induced second-harmonic generation (SHG) on a realistic metallic surface at atmospheric pressure. The surface is probed with a pulsed infrared laser beam and the SHG signal is monitored in reflection. For metallic silver, the SHG signal is found to be temperature dependent in the 25-120 degrees C range. The current accuracy of the method is +/-5 degrees C. Future work with platinum should permit the application of SHG thermometry to much higher surface temperatures.

  9. Chiral imaging of collagen by second-harmonic generation circular dichroism

    PubMed Central

    Lee, H.; Huttunen, M. J.; Hsu, K.-J.; Partanen, M.; Zhuo, G.-Y.; Kauranen, M.; Chu, S.-W.

    2013-01-01

    We provide evidence that the chirality of collagen can give rise to strong second-harmonic generation circular dichroism (SHG-CD) responses in nonlinear microscopy. Although chirality is an intrinsic structural property of collagen, most of the previous studies ignore that property. We demonstrate chiral imaging of individual collagen fibers by using a laser scanning microscope and type-I collagen from pig ligaments. 100% contrast level of SHG-CD is achieved with sub-micrometer spatial resolution. As a new contrast mechanism for imaging chiral structures in bio-tissues, this technique provides information about collagen morphology and three-dimensional orientation of collagen molecules. PMID:23761852

  10. Imaging morphodynamics of human blood cells in vivo with video-rate third harmonic generation microscopy

    PubMed Central

    Chen, Chien-Kuo; Liu, Tzu-Ming

    2012-01-01

    With a video-rate third harmonic generation (THG) microscopy system, we imaged the micro-circulation beneath the human skin without labeling. Not only the speed of circulation but also the morpho-hydrodynamics of blood cells can be analyzed. Lacking of nuclei, red blood cells (RBCs) shows typical parachute-like and hollow-core morphology under THG microscopy. Quite different from RBCs, every now and then, round and granule rich blood cells with strong THG contrast appear in circulation. The corresponding volume densities in blood, evaluated from their frequencies of appearance and the velocity of circulation, fall within the physiological range of human white blood cell counts. PMID:23162724

  11. Imaging morphodynamics of human blood cells in vivo with video-rate third harmonic generation microscopy.

    PubMed

    Chen, Chien-Kuo; Liu, Tzu-Ming

    2012-11-01

    With a video-rate third harmonic generation (THG) microscopy system, we imaged the micro-circulation beneath the human skin without labeling. Not only the speed of circulation but also the morpho-hydrodynamics of blood cells can be analyzed. Lacking of nuclei, red blood cells (RBCs) shows typical parachute-like and hollow-core morphology under THG microscopy. Quite different from RBCs, every now and then, round and granule rich blood cells with strong THG contrast appear in circulation. The corresponding volume densities in blood, evaluated from their frequencies of appearance and the velocity of circulation, fall within the physiological range of human white blood cell counts. PMID:23162724

  12. Third harmonic generation imaging for fast, label-free pathology of human brain tumors

    PubMed Central

    Kuzmin, N. V.; Wesseling, P.; Hamer, P. C. de Witt; Noske, D. P.; Galgano, G. D.; Mansvelder, H. D.; Baayen, J. C.; Groot, M. L.

    2016-01-01

    In brain tumor surgery, recognition of tumor boundaries is key. However, intraoperative assessment of tumor boundaries by the neurosurgeon is difficult. Therefore, there is an urgent need for tools that provide the neurosurgeon with pathological information during the operation. We show that third harmonic generation (THG) microscopy provides label-free, real-time images of histopathological quality; increased cellularity, nuclear pleomorphism, and rarefaction of neuropil in fresh, unstained human brain tissue could be clearly recognized. We further demonstrate THG images taken with a GRIN objective, as a step toward in situ THG microendoscopy of tumor boundaries. THG imaging is thus a promising tool for optical biopsies. PMID:27231629

  13. Ionization and high-order harmonic generation in aligned benzene by a short intense circularly polarized laser pulse

    SciTech Connect

    Baer, Roi; Neuhauser, Daniel; Zdanska, Petra R.; Moiseyev, Nimrod

    2003-10-01

    We present a first-principles study of ionization and high-order harmonic generation by benzene aligned in the polarization plane of a short circularly polarized laser pulse. Time-dependent density-functional theory within the adiabatic local-density approximation is employed to describe the 30 valence-electron dynamics in three dimensions. The multielectron approach enables us to study the effect of very strong laser fields, 10{sup 14}-10{sup 15} W cm{sup -2}, where multiple ionization and high-order harmonic generation interplay. Large ionization currents are formed, causing ionization of 1-4 electron charges, while strong high-order harmonic generation is observed. The well-known recollision mechanism of high-order harmonic generation plays a part for moderate laser intensities but is fully suppressed for strong laser fields. The harmonic generation spectra are characterized by two distinguishable plateaus, where the structure of the first plateau is dominated by the 6k{+-}1 (k=0,1,...) selection rule. The number of harmonics in the second plateau is insensitive to the duration of the pulse. The peaks appear in pairs or in threesomes, depending on the pulse duration.

  14. Dynamical origin of near- and below-threshold harmonic generation of Cs in an intense mid-infrared laser field

    PubMed Central

    Li, Peng-Cheng; Sheu, Yae-Lin; Laughlin, Cecil; Chu, Shih-I

    2015-01-01

    Near- and below-threshold harmonic generation provides a potential approach to generate vacuum-ultraviolet frequency comb. However, the dynamical origin of in these lower harmonics is less understood and largely unexplored. Here we perform an ab initio quantum study of the near- and below-threshold harmonic generation of caesium (Cs) atoms in an intense 3,600-nm mid-infrared laser field. Combining with a synchrosqueezing transform of the quantum time-frequency spectrum and an extended semiclassical analysis, the roles of multiphoton and multiple rescattering trajectories on the near- and below-threshold harmonic generation processes are clarified. We find that the multiphoton-dominated trajectories only involve the electrons scattered off the higher part of the combined atom-field potential followed by the absorption of many photons in near- and below-threshold regime. Furthermore, only the near-resonant below-threshold harmonic is exclusive to exhibit phase locked features. Our results shed light on the dynamic origin of the near- and below-threshold harmonic generation. PMID:25990452

  15. Phase-matching analysis of high-order harmonics generated by truncated Bessel beams in the sub-10-fs regime

    SciTech Connect

    Altucci, C.; Bruzzese, R.; De Lisio, C.; Nisoli, M.; Priori, E.; Stagira, S.; Pascolini, M.; Poletto, L.; Villoresi, P.; Tosa, V.; Midorikawa, K.

    2003-09-01

    We describe a very simple physical model that allows the analysis of high-order harmonic generation in gases when the pumping laser beam has an intensity profile that is not Gaussian but truncated Bessel. This is the typical experimental condition when sub-10-fs pump-laser pulses, generated by the hollow fiber compression technique, are used. This model is based on the analysis of the phase-matching conditions for the harmonic generation process revisited in view of the new spatial mode of the fundamental beam. In particular, the role of the atomic dipole phase and the geometric phase terms are evidenced both for harmonics generated in the plateau and in the cutoff spectral regions. The influence of dispersion introduced by free electrons produced by laser ionization has also been discussed in some detail. Spatial patterns of far-field harmonics are then obtained by means of a simplified algorithm which allows one to avoid the numerical integration of the harmonic beam propagation equation. Experimental spatial distributions and divergence angles of high-order harmonics generated in Ne with 7-fs titanium-sapphire pulses are compared with numerical simulations in various experimental conditions. The agreement between measurements and calculated results is found to be very satisfactory.

  16. Polarization second harmonic generation microscopy provides quantitative enhanced molecular specificity for tissue diagnostics.

    PubMed

    Kumar, Rajesh; Grønhaug, Kirsten M; Romijn, Elisabeth I; Finnøy, Andreas; Davies, Catharina L; Drogset, Jon O; Lilledahl, Magnus B

    2015-09-01

    Due to specific structural organization at the molecular level, several biomolecules (e.g., collagen, myosin etc.) which are strong generators of second harmonic generation (SHG) signals, exhibit unique responses depending on the polarization of the excitation light. By using the polarization second harmonic generation (p-SHG) technique, the values of the second order susceptibility components can be used to differentiate the types of molecule, which cannot be done by the use of a standard SHG intensity image. In this report we discuss how to implement p-SHG on a commercial multiphoton microscope and overcome potential artifacts in susceptibility (χ) image. Furthermore we explore the potential of p-SHG microscopy by applying the technique to different types of tissue in order to determine corresponding reference values of the ratio of second-order χ tensor elements. These values may be used as a bio-marker to detect any structural alterations in pathological tissue for diagnostic purposes. The SHG intensity image (red) in (a) shows the distribution of collagen fibers in ovary tissue but cannot determine the type of collagen fiber. However, the histogram distribution (b) for the values of the χ tensor element ratio can be used to quantitatively identify the types of collagen fibers.

  17. Scaling high-order harmonic generation from laser-solid interactions to ultrahigh intensity.

    PubMed

    Dollar, F; Cummings, P; Chvykov, V; Willingale, L; Vargas, M; Yanovsky, V; Zulick, C; Maksimchuk, A; Thomas, A G R; Krushelnick, K

    2013-04-26

    Coherent x-ray beams with a subfemtosecond (<10(-15)  s) pulse duration will enable measurements of fundamental atomic processes in a completely new regime. High-order harmonic generation (HOHG) using short pulse (<100  fs) infrared lasers focused to intensities surpassing 10(18)  W cm(-2) onto a solid density plasma is a promising means of generating such short pulses. Critical to the relativistic oscillating mirror mechanism is the steepness of the plasma density gradient at the reflection point, characterized by a scale length, which can strongly influence the harmonic generation mechanism. It is shown that for intensities in excess of 10(21)  W cm(-2) an optimum density ramp scale length exists that balances an increase in efficiency with a growth of parametric plasma wave instabilities. We show that for these higher intensities the optimal scale length is c/ω0, for which a variety of HOHG properties are optimized, including total conversion efficiency, HOHG divergence, and their power law scaling. Particle-in-cell simulations show striking evidence of the HOHG loss mechanism through parametric instabilities and relativistic self-phase modulation, which affect the produced spectra and conversion efficiency.

  18. Scaling high-order harmonic generation from laser-solid interactions to ultrahigh intensity.

    PubMed

    Dollar, F; Cummings, P; Chvykov, V; Willingale, L; Vargas, M; Yanovsky, V; Zulick, C; Maksimchuk, A; Thomas, A G R; Krushelnick, K

    2013-04-26

    Coherent x-ray beams with a subfemtosecond (<10(-15)  s) pulse duration will enable measurements of fundamental atomic processes in a completely new regime. High-order harmonic generation (HOHG) using short pulse (<100  fs) infrared lasers focused to intensities surpassing 10(18)  W cm(-2) onto a solid density plasma is a promising means of generating such short pulses. Critical to the relativistic oscillating mirror mechanism is the steepness of the plasma density gradient at the reflection point, characterized by a scale length, which can strongly influence the harmonic generation mechanism. It is shown that for intensities in excess of 10(21)  W cm(-2) an optimum density ramp scale length exists that balances an increase in efficiency with a growth of parametric plasma wave instabilities. We show that for these higher intensities the optimal scale length is c/ω0, for which a variety of HOHG properties are optimized, including total conversion efficiency, HOHG divergence, and their power law scaling. Particle-in-cell simulations show striking evidence of the HOHG loss mechanism through parametric instabilities and relativistic self-phase modulation, which affect the produced spectra and conversion efficiency. PMID:23679739

  19. Concept for power scaling second harmonic generation using a cascade of nonlinear crystals.

    PubMed

    Hansen, A K; Tawfieq, M; Jensen, O B; Andersen, P E; Sumpf, B; Erbert, G; Petersen, P M

    2015-06-15

    Within the field of high-power second harmonic generation (SHG), power scaling is often hindered by adverse crystal effects such as thermal dephasing arising from the second harmonic (SH) light, which imposes limits on the power that can be generated in many crystals. Here we demonstrate a concept for efficient power scaling of single-pass SHG beyond such limits using a cascade of nonlinear crystals, in which the first crystal is chosen for high nonlinear efficiency and the subsequent crystal(s) are chosen for power handling ability. Using this highly efficient single-pass concept, we generate 3.7 W of continuous-wave diffraction-limited (M(2)=1.25) light at 532 nm from 9.5 W of non-diffraction-limited (M(2)=7.7) light from a tapered laser diode, while avoiding significant thermal effects. Besides constituting the highest SH power yet achieved using a laser diode, this demonstrates that the concept successfully combines the high efficiency of the first stage with the good power handling properties of the subsequent stages. The concept is generally applicable and can be expanded with more stages to obtain even higher efficiency, and extends also to other combinations of nonlinear media suitable for other wavelengths.

  20. High efficiency fourth-harmonic generation from nanosecond fiber master oscillator power amplifier

    NASA Astrophysics Data System (ADS)

    Mu, Xiaodong; Steinvurzel, Paul; Rose, Todd S.; Lotshaw, William T.; Beck, Steven M.; Clemmons, James H.

    2016-03-01

    We demonstrate high power, deep ultraviolet (DUV) conversion to 266 nm through frequency quadrupling of a nanosecond pulse width 1064 nm fiber master oscillator power amplifier (MOPA). The MOPA system uses an Yb-doped double-clad polarization-maintaining large mode area tapered fiber as the final gain stage to generate 0.5-mJ, 10 W, 1.7- ns single mode pulses at a repetition rate of 20 kHz with measured spectral bandwidth of 10.6 GHz (40 pm), and beam qualities of Mx 2=1.07 and My 2=1.03, respectively. Using LBO and BBO crystals for the second-harmonic generation (SHG) and fourth-harmonic generation (FHG), we have achieved 375 μJ (7.5 W) and 92.5 μJ (1.85 W) at wavelengths of 532 nm and 266 nm, respectively. To the best of our knowledge these are the highest narrowband infrared, green and UV pulse energies obtained to date from a fully spliced fiber amplifier. We also demonstrate high efficiency SHG and FHG with walk-off compensated (WOC) crystal pairs and tightly focused pump beam. An SHG efficiency of 75%, FHG efficiency of 47%, and an overall efficiency of 35% from 1064 nm to 266 nm are obtained.

  1. Generation of vacuum ultraviolet radiation by intracavity high-harmonic generation toward state detection of single trapped ions

    NASA Astrophysics Data System (ADS)

    Wakui, Kentaro; Hayasaka, Kazuhiro; Ido, Tetsuya

    2014-12-01

    Vacuum ultraviolet (VUV) radiation around 159 nm is obtained toward direct excitation of a single trapped ion. An efficient fluoride-based VUV output coupler is employed for intracavity high-harmonic generation of a Ti:S oscillator. Using this coupler, where we measured its reflectance to be about 90 %, an average power reaching 6.4 W is coupled out from a modest fundamental power of 650 mW. When a single comb component out of 1.9 10 teeth is resonant to the atomic transition, 100s of fluorescence photons per second will be detectable under a realistic condition.

  2. Multimodal two-photon imaging using a second harmonic generation-specific dye

    PubMed Central

    Nuriya, Mutsuo; Fukushima, Shun; Momotake, Atsuya; Shinotsuka, Takanori; Yasui, Masato; Arai, Tatsuo

    2016-01-01

    Second harmonic generation (SHG) imaging can be used to visualize unique biological phenomena, but currently available dyes limit its application owing to the strong fluorescent signals that they generate together with SHG. Here we report the first non-fluorescent and membrane potential-sensitive SHG-active organic dye Ap3. Ap3 is photostable and generates SH signals at the plasma membrane with virtually no fluorescent signals, in sharp contrast to the previously used fluorescent dye FM4-64. When tested in neurons, Ap3-SHG shows linear membrane potential sensitivity and fast responses to action potentials, and also shows significantly reduced photodamage compared with FM4-64. The SHG-specific nature of Ap3 allows simultaneous and completely independent imaging of SHG signals and fluorescent signals from various reporter molecules, including markers of cellular organelles and intracellular calcium. Therefore, this SHG-specific dye enables true multimodal two-photon imaging in biological samples. PMID:27156702

  3. High gain durable anti-reflective coating

    DOEpatents

    Maghsoodi, Sina; Brophy, Brenor L.; Colson, Thomas E.; Gonsalves, Peter R.; Abrams, Ze'ev R.

    2016-07-26

    Disclosed herein are polysilsesquioxane-based anti-reflective coating (ARC) compositions, methods of preparation, and methods of deposition on a substrate. In one embodiment, the polysilsesquioxane of this disclosure is prepared in a two-step process of acid catalyzed hydrolysis of organoalkoxysilane followed by addition of tetralkoxysilane that generates silicone polymers with >40 mol % silanol based on Si-NMR. These high silanol siloxane polymers are stable and have a long shelf-life in polar organic solvents at room temperature. Also disclosed are low refractive index ARC made from these compositions with and without additives such as porogens, templates, thermal radical initiator, photo radical initiators, crosslinkers, Si--OH condensation catalyst and nano-fillers. Also disclosed are methods and apparatus for applying coatings to flat substrates including substrate pre-treatment processes, coating processes and coating curing processes including skin-curing using hot-air knives. Also disclosed are coating compositions and formulations for highly tunable, durable, highly abrasion-resistant functionalized anti-reflective coatings.

  4. Modular approach to achieving the next-generation X-ray light source

    NASA Astrophysics Data System (ADS)

    Biedron, S. G.; Milton, S. V.; Freund, H. P.

    2001-12-01

    A modular approach to the next-generation light source is described. The "modules" include photocathode, radio-frequency, electron guns and their associated drive-laser systems, linear accelerators, bunch-compression systems, seed laser systems, planar undulators, two-undulator harmonic generation schemes, high-gain harmonic generation systems, nonlinear higher harmonics, and wavelength shifting. These modules will be helpful in distributing the next-generation light source to many more laboratories than the current single-pass, high-gain free-electron laser designs permit, due to both monetary and/or physical space constraints.

  5. A novel intravital multi-harmonic generation microscope for early diagnosis of oral cancer

    NASA Astrophysics Data System (ADS)

    Cheng, Yu-Hsiang; Lin, Chih-Feng; Shih, Ting-Fang; Sun, Chi-Kuang

    2013-03-01

    Oral cancer is one of the most frequently diagnosed human cancers and leading causes of cancer death all over the world, but the prognosis and overall survival rate are still poor because of delay in diagnosis and lack of early intervention. The failure of early diagnosis is due to insufficiency of proper diagnostic and screening tools and most patients are reluctant to undergo biopsy. Optical virtual biopsy techniques, for imaging cells and tissues at microscopic details capable of differentiating benign from malignant lesions non-invasively, are thus highly desirable. A novel multi-harmonic generation microscope, excited by a 1260 nm Cr:forsterite laser, with second and third harmonic signals demonstrating collagen fiber distribution and cell morphology in a sub-micron resolution, was developed for clinical use. To achieve invivo observation inside the human oral cavity, a small objective probe with a suction capability was carefully designed for patients' comfort and stability. By remotely changing its focus point, the same objective can image the mucosa surface with a low magnification, illuminated by side light-emitting diodes, with a charge-coupled device (CCD) for site location selection before the harmonic generation biopsy was applied. Furthermore, the slow galvanometer mirror and the fast resonant mirror provide a 30 fps frame rate for high-speed real-time observation and the z-motor of this system is triggered at the same rate to provide fast 3D scanning, again ensuring patients' comfort. Focusing on the special cytological and morphological changes of the oral epithelial cells, our preliminary result disclosed excellent consistency with traditional histopathology studies.

  6. Investigation of the Higher Harmonic Lamb Wave Generation in Hyperelastic Isotropic Material

    NASA Astrophysics Data System (ADS)

    Rauter, Natalie; Lammering, Rolf

    Micro-structural damages, such as micro-cracks and voids, give locally rise to stresses and may initiate subsequent failure of structural components. Therefore, the development of methods for the detection of microstructural damage and the observation of their growth is an important and ongoing area of research, especially for thin-walled structures. The proposed method for the detection is based on the nonlinearity caused by the micro-structural damages. Lamb waves are generated which induce simultaneously higher harmonic modes due the inherent nonlinearity. For detailed investigations, numerical simulations are essential. In this work, the nonlinearity is modeled by the material law, which is based on the Neo- Hookean and Mooney-Rivlin material models. In contrast to previous studies, which used third order elastic coefficients, these hyperelastic material models are widely accepted, frequently used, and implemented in commonly available FEM software. In the numerical investigations, Lamb waves are generated in a thin-walled aluminum plate with windowed sine burst signals. Due to the nonlinearity in the material law, the waves are not only observed at the excitation frequency, but also at higher harmonic frequencies. Excitation at especially selected frequencies evoke the cumulative effect, and thus gives rise to the amplitudes of the higher harmonics. Comparing the S1-S2 and S2-S4 mode pairs clearly show the higher sensitivity of the latter to the material nonlinearity. This matches with previous published experimental results. Finally, it is shown that the results obtained agree qualitatively well with numerical analyses, in which the micro-structural damages are modeled directly by a respective finite element discretization.

  7. Nonlinear generation of harmonics through the interaction of an internal wave beam with a model oceanic pycnocline

    NASA Astrophysics Data System (ADS)

    Diamessis, P. J.; Wunsch, S.; Delwiche, I.; Richter, M. P.

    2014-06-01

    The interaction of an internal wave beam (IWB) with an idealized oceanic pycnocline is examined using two-dimensional fully nonlinear direct numerical simulations based on a spectral multidomain penalty method in the vertical direction. The phenomenon of focus is the nonlinear generation of harmonics. A total of 24 simulations have been performed, varying the normalized pycnocline thickness and the ratio of peak pycnocline Brunt-Väisälä frequency to that of the stratified lower layer. Harmonics at the point of IWB entry into the pycnocline increase in amplitude and number with a measure of the maximum gradient of the Brunt-Väisälä frequency, suggesting refraction as an important factor in harmonic generation. Among the simulations performed, two distinct limits of pycnocline thickness are identified. For thin pynoclines, whose thickness is 10% of the incident IWB's horizontal wavelength, harmonics trapped within the pycnocline have maximum amplitude when their frequency and wavenumber match those of the natural pycnocline interfacial wave mode. Results in this case are compared with weakly nonlinear theory for harmonic generation by plane wave refraction. For thicker pycnoclines, whose thickness is equal the incident IWB's horizontal wavelength, IWB refraction results in harmonic generation at multiple locations in addition to pycnocline entry, giving rise to complex flow structure inside the pycnocline.

  8. Self-Consistent Calculation of Half-Harmonics Emission Generated by the Two-Plasmon-Decay Instability

    NASA Astrophysics Data System (ADS)

    Zhang, J.; Myatt, J. F.; Maximov, A. V.; Short, R. W.; Dubois, D. F.; Russell, D. A.; Vu, H. X.

    2014-10-01

    Half-harmonics emission can be used as an effective diagnostic tool for the two-plasmon-decay (TPD) instability. However, interpretation of the half-harmonics spectrum is difficult because of its complicated generation mechanism. We have developed a code that can calculate half-harmonics emission self-consistently with the TPD instability. The results would be useful to interpret experimental data and help design experiments. This material is based upon work supported by the Department of Energy National Nuclear Security Administration under Award Number DE-NA0001944.

  9. Field localization and enhancement of phase-locked second- and third-order harmonic generation in absorbing semiconductor cavities

    SciTech Connect

    Roppo, V.; Cojocaru, C.; Trull, J.; Vilaseca, R.; Raineri, F.; Halioua, Y.; Raj, R.; Sagnes, I.; D'Aguanno, G.; Scalora, M.

    2009-10-15

    We predict and experimentally observe the enhancement by three orders of magnitude of phase mismatched second and third harmonic generation in a GaAs cavity at 650 and 433 nm, respectively, well above the absorption edge. Phase locking between the pump and the harmonics changes the effective dispersion of the medium and inhibits absorption. Despite hostile conditions the harmonics resonate inside the cavity and become amplified leading to relatively large conversion efficiencies. Field localization thus plays a pivotal role despite the presence of absorption, and ushers in a new class of semiconductor-based devices in the visible and uv ranges.

  10. Parametric Harmonic Generation as a Probe of Unconstrained Spin Magnetization Precession in the Shallow Barrier Limit.

    PubMed

    Capua, Amir; Rettner, Charles; Parkin, Stuart S P

    2016-01-29

    We study the parametric excitation of high orders of magnetization precession in ultrathin films having perpendicular magnetic anisotropy. We observe that for a given driving field amplitude the harmonic generation can be increased by lowering the barrier with the application of an in-plane magnetic field in the manner of the Smit-Beljers effect. In this effect, the magnetic stiffness is reduced not by lowering the magnitude of the magnetic field upon which the spins precess, but rather by effectively releasing the field's "anchoring" point. This results in a shallow energy barrier where the electrons' spin is locally unconstrained. While the observation is unveiled in the form of nonlinear high harmonic generation, we believe that the physics whereby the barrier is suppressed by an external magnetic field may apply to other phenomena associated with ultrathin films. In these cases, such unconstrained motion may serve as a sensitive probe of the torques associated with proximate spin currents. Moreover, our approach may be used as a model system for the study of phase transitions in the field of nonlinear dynamics.

  11. Electrical control of second-harmonic generation in a WSe2 monolayer transistor

    NASA Astrophysics Data System (ADS)

    Seyler, Kyle L.; Schaibley, John R.; Gong, Pu; Rivera, Pasqual; Jones, Aaron M.; Wu, Sanfeng; Yan, Jiaqiang; Mandrus, David G.; Yao, Wang; Xu, Xiaodong

    2015-05-01

    Nonlinear optical frequency conversion, in which optical fields interact with a nonlinear medium to produce new field frequencies, is ubiquitous in modern photonic systems. However, the nonlinear electric susceptibilities that give rise to such phenomena are often challenging to tune in a given material and, so far, dynamical control of optical nonlinearities remains confined to research laboratories as a spectroscopic tool. Here, we report a mechanism to electrically control second-order optical nonlinearities in monolayer WSe2, an atomically thin semiconductor. We show that the intensity of second-harmonic generation at the A-exciton resonance is tunable by over an order of magnitude at low temperature and nearly a factor of four at room temperature through electrostatic doping in a field-effect transistor. Such tunability arises from the strong exciton charging effects in monolayer semiconductors, which allow for exceptional control over the oscillator strengths at the exciton and trion resonances. The exciton-enhanced second-harmonic generation is counter-circularly polarized to the excitation laser due to the combination of the two-photon and one-photon valley selection rules, which have opposite helicity in the monolayer. Our study paves the way towards a new platform for chip-scale, electrically tunable nonlinear optical devices based on two-dimensional semiconductors.

  12. High-order-harmonic generation in molecular sequential double ionization by intense circularly polarized laser pulses

    NASA Astrophysics Data System (ADS)

    Yuan, Kai-Jun; Lu, Huizhong; Bandrauk, André D.

    2015-08-01

    We present effects of electron energy transfer by electron collisions on high-order-harmonic generation (HHG) in molecular sequential double ionization by intense circularly polarized laser pulses. Results from numerical solutions of time-dependent Schrödinger equations for extended (large internuclear distance) H2 where electrons are entangled and hence delocalized by exchange show that HHG with cutoff energy up to Ip+24 Up can be obtained, where Ip is the molecule ionization potential and Up=I0/4 ω02 (in atomic units) is the ponderomotive energy for pulse intensity I0 and frequency ω0. A time-frequency analysis is employed to identify electron collisions for the generation of harmonics. Extended HHG arises from electron energy exchange, which agrees well with the prediction of a classical two electron collision model. Results for nonsymmetric HHe+ where initially electrons are localized on He are also compared and confirm the role of initial electron delocalization via entanglement for obtaining extended HHG plateaus.

  13. Absolute polarity determination of teeth cementum by phase sensitive second harmonic generation microscopy.

    PubMed

    Aboulfadl, Hanane; Hulliger, Jürg

    2015-10-01

    The absolute sign of local polarity in relation to the biological growth direction has been investigated for teeth cementum using phase sensitive second harmonic generation microscopy (PS-SHGM) and a crystal of 2-cyclooctylamino-5-nitropyridine (COANP) as a nonlinear optic (NLO) reference material. A second harmonic generation (SHG) response was found in two directions of cementum: radial (acellular extrinsic fibers that are oriented more or less perpendicular to the root surface) and circumferential (cellular intrinsic fibers that are oriented more or less parallel to the surface). A mono-polar state was demonstrated for acellular extrinsic cementum. However, along the different parts of cementum in circumferential direction, two corresponding domains were observed featuring an opposite sign of polarity indicative for a bi-polar microscopic state of cellular intrinsic cementum. The phase information showed that the orientation of radial collagen fibrils of cementum is regularly organized with the donor (D) groups pointing to the surface. Circumferential collagen molecules feature orientational disorder and are oriented up and down in random manner showing acceptor or donor groups at the surface of cementum. Considering that the cementum continues to grow in thickness throughout life, we can conclude that the cementum is growing circumferentially in two opposite directions and radially in one direction. A Markov chain type model for polarity formation in the direction of growth predicts D-groups preferably appearing at the fiber front.

  14. Second harmonic generation in nanoscale films of transition metal dichalcogenide: Accounting for multipath interference

    NASA Astrophysics Data System (ADS)

    Kudryavtsev, A. V.; Lavrov, S. D.; Shestakova, A. P.; Kulyuk, L. L.; Mishina, E. D.

    2016-09-01

    The transfer matrix method has been widely used to calculate wave propagation through the layered structures consisting entirely of either linear or nonlinear optical materials. In the present work, we develop the transfer matrix method for structures consisting of alternating layers of linear and nonlinear optical materials. The result is presented in a form that allows one to directly substitute the values of material constants, refractive index and absorption coefficient, into the expressions describing the second harmonic generation (SHG) field. The model is applied to the calculation of second harmonic (SH) field generated in nano-thin layers of transition metal dichalcogenides exfoliated on top of silicon oxide/silicon Fabry-Perot cavity. These structures are intensively studied both in view of their unique properties and perspective applications. A good agreement between experimental and numerical results can be achieved by small modification of optical constants, which may arise in an experiment due to a strong electric field of an incident focused pump laser beam. By considering the SHG effect, this paper completes the series of works describing the role of Fabry-Perot cavity in different optical effects (optical reflection, photoluminescence and Raman scattering) in 2D semiconductors that is extremely important for characterization of these unique materials.

  15. Parametric Harmonic Generation as a Probe of Unconstrained Spin Magnetization Precession in the Shallow Barrier Limit.

    PubMed

    Capua, Amir; Rettner, Charles; Parkin, Stuart S P

    2016-01-29

    We study the parametric excitation of high orders of magnetization precession in ultrathin films having perpendicular magnetic anisotropy. We observe that for a given driving field amplitude the harmonic generation can be increased by lowering the barrier with the application of an in-plane magnetic field in the manner of the Smit-Beljers effect. In this effect, the magnetic stiffness is reduced not by lowering the magnitude of the magnetic field upon which the spins precess, but rather by effectively releasing the field's "anchoring" point. This results in a shallow energy barrier where the electrons' spin is locally unconstrained. While the observation is unveiled in the form of nonlinear high harmonic generation, we believe that the physics whereby the barrier is suppressed by an external magnetic field may apply to other phenomena associated with ultrathin films. In these cases, such unconstrained motion may serve as a sensitive probe of the torques associated with proximate spin currents. Moreover, our approach may be used as a model system for the study of phase transitions in the field of nonlinear dynamics. PMID:26871356

  16. Absolute polarity determination of teeth cementum by phase sensitive second harmonic generation microscopy.

    PubMed

    Aboulfadl, Hanane; Hulliger, Jürg

    2015-10-01

    The absolute sign of local polarity in relation to the biological growth direction has been investigated for teeth cementum using phase sensitive second harmonic generation microscopy (PS-SHGM) and a crystal of 2-cyclooctylamino-5-nitropyridine (COANP) as a nonlinear optic (NLO) reference material. A second harmonic generation (SHG) response was found in two directions of cementum: radial (acellular extrinsic fibers that are oriented more or less perpendicular to the root surface) and circumferential (cellular intrinsic fibers that are oriented more or less parallel to the surface). A mono-polar state was demonstrated for acellular extrinsic cementum. However, along the different parts of cementum in circumferential direction, two corresponding domains were observed featuring an opposite sign of polarity indicative for a bi-polar microscopic state of cellular intrinsic cementum. The phase information showed that the orientation of radial collagen fibrils of cementum is regularly organized with the donor (D) groups pointing to the surface. Circumferential collagen molecules feature orientational disorder and are oriented up and down in random manner showing acceptor or donor groups at the surface of cementum. Considering that the cementum continues to grow in thickness throughout life, we can conclude that the cementum is growing circumferentially in two opposite directions and radially in one direction. A Markov chain type model for polarity formation in the direction of growth predicts D-groups preferably appearing at the fiber front. PMID:26297858

  17. Genetic algorithm applied to the optimization of quantum cascade lasers with second harmonic generation

    SciTech Connect

    Gajić, A.; Radovanović, J. Milanović, V.; Indjin, D.; Ikonić, Z.

    2014-02-07

    A computational model for the optimization of the second order optical nonlinearities in GaInAs/AlInAs quantum cascade laser structures is presented. The set of structure parameters that lead to improved device performance was obtained through the implementation of the Genetic Algorithm. In the following step, the linear and second harmonic generation power were calculated by self-consistently solving the system of rate equations for carriers and photons. This rate equation system included both stimulated and simultaneous double photon absorption processes that occur between the levels relevant for second harmonic generation, and material-dependent effective mass, as well as band nonparabolicity, were taken into account. The developed method is general, in the sense that it can be applied to any higher order effect, which requires the photon density equation to be included. Specifically, we have addressed the optimization of the active region of a double quantum well In{sub 0.53}Ga{sub 0.47}As/Al{sub 0.48}In{sub 0.52}As structure and presented its output characteristics.

  18. Texture analysis applied to second harmonic generation image data for ovarian cancer classification.

    PubMed

    Wen, Bruce L; Brewer, Molly A; Nadiarnykh, Oleg; Hocker, James; Singh, Vikas; Mackie, Thomas R; Campagnola, Paul J

    2014-09-01

    Remodeling of the extracellular matrix has been implicated in ovarian cancer. To quantitate the remodeling, we implement a form of texture analysis to delineate the collagen fibrillar morphology observed in second harmonic generation microscopy images of human normal and high grade malignant ovarian tissues. In the learning stage, a dictionary of “textons”—frequently occurring texture features that are identified by measuring the image response to a filter bank of various shapes, sizes, and orientations—is created. By calculating a representative model based on the texton distribution for each tissue type using a training set of respective second harmonic generation images, we then perform classification between images of normal and high grade malignant ovarian tissues. By optimizing the number of textons and nearest neighbors, we achieved classification accuracy up to 97% based on the area under receiver operating characteristic curves (true positives versus false positives). The local analysis algorithm is a more general method to probe rapidly changing fibrillar morphologies than global analyses such as FFT. It is also more versatile than other texture approaches as the filter bank can be highly tailored to specific applications (e.g., different disease states) by creating customized libraries based on common image features. PMID:26296156

  19. Vacuum high-harmonic generation in the shock regime and photon-photon scattering dynamics

    NASA Astrophysics Data System (ADS)

    King, B.; Böhl, P.; Ruhl, H.

    2016-02-01

    The presence of charged quantum virtual states permits a nonlinear self-interaction of the electromagnetic field in vacuum. This interaction can be described as real photon-photon scattering. This effect has been calculated for the case of colliding plane waves, when the centre- of-mass energy is much less than the electron rest energy. The quantum effect is included in the classical electromagnetic field equations of motion by a standard effective approach based upon a weak-field expansion of the Heisenberg-Euler Lagrangian. Solving for the resultant electromagnetic field indicates a signal for real photon-photon scattering when the plane waves overlap, which can be significantly larger than the usually-considered asymptotic values that reach detectors. By considering arbitrary numbers of four- and six-photon scattering, the process of vacuum higher harmonic generation has been studied both analytically and numerically. A route to prolific harmonic generation is identified that does not depend on field strengths being necessarily close to the Schwinger limit. The resulting vacuum electromagnetic shock wave has been studied and a nonlinear shock parameter identified.

  20. Quantitative second-harmonic generation imaging to detect osteogenesis imperfecta in human skin samples

    NASA Astrophysics Data System (ADS)

    Adur, J.; Ferreira, A. E.; D'Souza-Li, L.; Pelegati, V. B.; de Thomaz, A. A.; Almeida, D. B.; Baratti, M. O.; Carvalho, H. F.; Cesar, C. L.

    2012-03-01

    Osteogenesis Imperfecta (OI) is a genetic disorder that leads to bone fractures due to mutations in the Col1A1 or Col1A2 genes that affect the primary structure of the collagen I chain with the ultimate outcome in collagen I fibrils that are either reduced in quantity or abnormally organized in the whole body. A quick test screening of the patients would largely reduce the sample number to be studied by the time consuming molecular genetics techniques. For this reason an assessment of the human skin collagen structure by Second Harmonic Generation (SHG) can be used as a screening technique to speed up the correlation of genetics/phenotype/OI types understanding. In the present work we have used quantitative second harmonic generation (SHG) imaging microscopy to investigate the collagen matrix organization of the OI human skin samples comparing with normal control patients. By comparing fibril collagen distribution and spatial organization, we calculated the anisotropy and texture patterns of this structural protein. The analysis of the anisotropy was performed by means of the two-dimensional Discrete Fourier Transform and image pattern analysis with Gray-Level Co-occurrence Matrix (GLCM). From these results, we show that statistically different results are obtained for the normal and disease states of OI.

  1. Modified Perfect Harmonics Cancellation Control of a Grid Interfaced SPV Power Generation

    NASA Astrophysics Data System (ADS)

    Singh, B.; Shahani, D. T.; Verma, A. K.

    2015-03-01

    This paper deals with a grid interfaced solar photo voltaic (SPV) power generating system with modified perfect harmonic cancellation (MPHC) control for power quality improvement in terms of mitigation of the current harmonics, power factor correction, control of point of common coupling (PCC) voltage with reactive power compensation and load balancing in a three phase distribution system. The proposed grid interfaced SPV system consists of a SPV array, a dc-dc boost converter and a voltage source converter (VSC) used for the compensation of other connected linear and nonlinear loads at PCC. The reference grid currents are estimated using MPHC method and control signals are derived by using pulse width modulation (PWM) current controller of VSC. The SPV power is fed to the common dc bus of VSC and dc-dc boost converter using maximum power point tracking (MPPT). The dc link voltage of VSC is regulated by using dc voltage proportional integral (PI) controller. The analysis of the proposed SPV power generating system is carried out under dc/ac short circuit and severe SPV-SX and SPV-TX intrusion.

  2. Electrical control of second-harmonic generation in a WSe2 monolayer transistor

    SciTech Connect

    Seyler, Kyle L.; Schaibley, John R.; Gong, Pu; Rivera, Pasqual; Jones, Aaron M.; Wu, Sanfeng; Yan, Jiaqiang; Mandrus, David G.; Yao, Wang; Xu, Xiaodong

    2015-04-20

    Nonlinear optical frequency conversion, in which optical fields interact with a nonlinear medium to produce new field frequencies, is ubiquitous in modern photonic systems. However, the nonlinear electric susceptibilities that give rise to such phenomena are often challenging to tune in a given material and, so far, dynamical control of optical nonlinearities remains confined to research laboratories as a spectroscopic tool. In this paper, we report a mechanism to electrically control second-order optical nonlinearities in monolayer WSe2, an atomically thin semiconductor. We show that the intensity of second-harmonic generation at the A-exciton resonance is tunable by over an order of magnitude at low temperature and nearly a factor of four at room temperature through electrostatic doping in a field-effect transistor. Such tunability arises from the strong exciton charging effects in monolayer semiconductors, which allow for exceptional control over the oscillator strengths at the exciton and trion resonances. The exciton-enhanced second-harmonic generation is counter-circularly polarized to the excitation laser due to the combination of the two-photon and one-photon valley selection rules, which have opposite helicity in the monolayer. Finally, our study paves the way towards a new platform for chip-scale, electrically tunable nonlinear optical devices based on two-dimensional semiconductors.

  3. Electrical control of second-harmonic generation in a WSe2 monolayer transistor

    DOE PAGES

    Seyler, Kyle L.; Schaibley, John R.; Gong, Pu; Rivera, Pasqual; Jones, Aaron M.; Wu, Sanfeng; Yan, Jiaqiang; Mandrus, David G.; Yao, Wang; Xu, Xiaodong

    2015-04-20

    Nonlinear optical frequency conversion, in which optical fields interact with a nonlinear medium to produce new field frequencies, is ubiquitous in modern photonic systems. However, the nonlinear electric susceptibilities that give rise to such phenomena are often challenging to tune in a given material and, so far, dynamical control of optical nonlinearities remains confined to research laboratories as a spectroscopic tool. In this paper, we report a mechanism to electrically control second-order optical nonlinearities in monolayer WSe2, an atomically thin semiconductor. We show that the intensity of second-harmonic generation at the A-exciton resonance is tunable by over an order ofmore » magnitude at low temperature and nearly a factor of four at room temperature through electrostatic doping in a field-effect transistor. Such tunability arises from the strong exciton charging effects in monolayer semiconductors, which allow for exceptional control over the oscillator strengths at the exciton and trion resonances. The exciton-enhanced second-harmonic generation is counter-circularly polarized to the excitation laser due to the combination of the two-photon and one-photon valley selection rules, which have opposite helicity in the monolayer. Finally, our study paves the way towards a new platform for chip-scale, electrically tunable nonlinear optical devices based on two-dimensional semiconductors.« less

  4. Texture analysis applied to second harmonic generation image data for ovarian cancer classification

    NASA Astrophysics Data System (ADS)

    Wen, Bruce L.; Brewer, Molly A.; Nadiarnykh, Oleg; Hocker, James; Singh, Vikas; Mackie, Thomas R.; Campagnola, Paul J.

    2014-09-01

    Remodeling of the extracellular matrix has been implicated in ovarian cancer. To quantitate the remodeling, we implement a form of texture analysis to delineate the collagen fibrillar morphology observed in second harmonic generation microscopy images of human normal and high grade malignant ovarian tissues. In the learning stage, a dictionary of "textons"-frequently occurring texture features that are identified by measuring the image response to a filter bank of various shapes, sizes, and orientations-is created. By calculating a representative model based on the texton distribution for each tissue type using a training set of respective second harmonic generation images, we then perform classification between images of normal and high grade malignant ovarian tissues. By optimizing the number of textons and nearest neighbors, we achieved classification accuracy up to 97% based on the area under receiver operating characteristic curves (true positives versus false positives). The local analysis algorithm is a more general method to probe rapidly changing fibrillar morphologies than global analyses such as FFT. It is also more versatile than other texture approaches as the filter bank can be highly tailored to specific applications (e.g., different disease states) by creating customized libraries based on common image features.

  5. Coupling CARS with multiphoton fluorescence and high harmonic generation imaging modalities using a femtosecond laser source

    NASA Astrophysics Data System (ADS)

    Chen, Hongtao; Slipchenko, Mikhail N.; Zhu, Jiabin; Buhman, Kimberly K.; Cheng, Ji-Xin

    2009-02-01

    Multimodal nonlinear optical imaging has opened new opportunities and becomes a powerful tool for imaging complex tissue samples with inherent 3D spatial resolution.. We present a robust and easy-to-operate approach to add the coherent anti-stokes Raman scattering (CARS) imaging modality to a widely used multiphoton microscope. The laser source composed of a Mai Tai femtosecond laser and an optical parametric oscillator (OPO) offers one-beam, two-beam and three-beam modalities. The Mai Tai output at 790 nm is split into two beams, with 80% of the power being used to pump the OPO. The idler output at 2036 nm from OPO is doubled using a periodically poled lithium niobate (PPLN) crystal. This frequency-doubled idler beam at 1018 nm is sent through a delay line and collinearly combined with the other Mai Tai beam for CARS imaging on a laser-scanning microscope. This Mai Tai beam is also used for multiphoton fluorescence and second harmonic generation (SHG) imaging. The signal output at 1290 nm from OPO is used for SHG and third-harmonic generation (THG) imaging. External detectors are installed for both forward and backward detection, whereas two internal lamda-scan detectors are employed for microspectroscopy analysis. This new system allows vibrationally resonant CARS imaging of lipid bodies, SHG imaging of collagen fibers, and multiphoton fluorescence analysis in fresh tissues. As a preliminary application, the effect of diacylglycerol acyltransferase 1 (DGAT1) deficiency on liver lipid metabolism in mice was investigated.

  6. Quantitative analysis of diseased horse tendons using Fourier-transform-second-harmonic generation imaging

    NASA Astrophysics Data System (ADS)

    Sivaguru, Mayandi; Durgam, Sushmitha; Ambekar, Raghu; Luedtke, David; Fried, Glenn; Stewart, Allison; Toussaint, Kimani C., Jr.

    2011-03-01

    Fourier transform-second-harmonic generation (FT-SHG) imaging is used to quantitatively assess the structural organization of collagen fibers in tendonitis-induced horse tendons. Fiber orientation, isotropy, and the ratio of forward to backward SHG signal (F/B ratio) are used to differentiate the fiber organization between the normal and diseased horse tendons. Each second-harmonic generation (SHG) image is divided into several smaller regions of interest (ROI) and the aforementioned quantitative metrics are calculated across the whole grid. ROIs are further labeled as dark (no or minimal presence of fibers), isotropic (random fiber organization), or anisotropic (regular fiber organization) regions. Results show that the normal tendon possesses minimal isotropic regions and small standard deviations in the histograms of orientation and F/B ratio, indicating an intact and highly regular fiber organization. However, the tendonitis-induced horse tendons possess higher number of dark and isotropic regions, and larger standard deviations of the measured parameters, suggesting significantly disoriented and disorganized collagen fibers. This type of quantification would be highly beneficial in diagnosing and determining the stage of tendonitis in clinical settings. Not limited to tendonitis, the technique could also be applied to other diseases that structurally affect collagen fibers. The advantage of FT-SHG over the conventional polarization microscopy is also discussed.

  7. Model for second-harmonic generation in glass optical fibers based on asymmetric photoelectron emission from defect sites.

    PubMed

    Anderson, D Z; Mizrahi, V; Sipe, J E

    1991-06-01

    We present a self-consistent calculation of anomalous second-harmonic generation in glass optical fibers. Quantum interference between multiphoton absorption processes leads to asymmetric photoelectric emission from defects, creating a spatially periodic space-charge electric field. The second harmonic is found to grow exponentially along the fiber, then saturate to a maximum value proportional to the square of the fundamental intensity. The predicted conversion efficiency is in reasonable agreement with experiments.

  8. Impact of Tidal-Stream Turbines on the Generation of the Higher Tidal Harmonics

    NASA Astrophysics Data System (ADS)

    Potter, Daniel; Ilic, Suzana; Folkard, Andrew

    2016-04-01

    The higher tidal harmonics result from the interaction of the astronomic tides with both themselves and each other through non-linear processes. In shallower waters such as those near the coast these non-linear processes become more significant and thus, so too do the higher tidal harmonics become more significant. The interaction of the tide with tidal-stream turbines (TSTs), through thrust and drag processes will be non-linear and as such will contribute to the generation of higher tidal harmonics, thus changing the nature of the tide downstream of the turbines. The change to the tide may potentially impact on the downstream energy resource (Robins et al. 2015) and sediment transport processes (Pingree & Griffiths 1979). This paper will present analytical results, which suggest that TSTs will impact on the generation of all higher harmonics but with odd overtides being impacted more than even overtides, the most important examples of which are the M6 and M4 tides respectively, which are the first odd and even overtides of the M2 tide. Change in phase and amplitude of the M6 tide by TSTs will distort the tide but will not cause an asymmetry between the flood and ebb of the tide. Change in the phase and amplitude of the M4 can not only distort the tide but also cause asymmetry. Hence any change to the M4 tide by the turbines is more significant, despite the magnitude of change to the M6 being greater. In order to gain a fuller understanding of the way in which TSTs change the tide downstream and the significance of any change for transport processes or energy resource, a numerical modelling study will be carried out, which will be presented in a future paper. Robins, P.E., Neill, S.P., Lewis, M. & Ward, S.L., 2015. Characterising the spatial and temporal variability of the tidal-stream energy resource over the northwest European shelf seas. Applied Energy, 147: 510-522. Pingree, R.D. & Griffiths, D.K., 1979. Sand transport paths around the British Isles resulting

  9. Synthesis of cervical tissue second harmonic generation images using Markov random field modeling.

    PubMed

    Yousefi, S; Kehtarnavaz, N; Gholipour, A

    2011-01-01

    This paper presents a statistical image modeling approach based on Markov random field to synthesize cervical tissue second harmonic generation (SHG) images. Binary images representing fiber and pore areas of the cervix tissue are first obtained from SHG images using an image processing pipeline consisting of noise removal, contrast enhancement and optimal thresholding. These binary images are modeled using a Markov random field whose parameters are estimated via the least squares method. The parameters are then used to synthesize fiber and pore areas of cervical tissue in the form of binary images. The effectiveness of the synthesis is demonstrated by reporting the classification outcome for two classes of cervical SHG images collected from mice at two different stages of normal pregnancy. The developed synthesis allows generation of realistic fiber and pore area binary images for cervical tissue studies.

  10. Conformation, orientation and interaction in molecular monolayers: A surface second harmonic and sum frequency generation study

    SciTech Connect

    Superfine, R.; Huang, J.Y.; Shen, Y.R.

    1988-12-01

    We have used sum frequency generation (SFG) to study the order in a silane monolayer before and after the deposition of a coadsorbed liquid crystal monolayer. We observe an increase in the order of the chain of the silane molecule induced by the interpenetration of the liquid crystal molecules. By using second harmonic generation (SHG) and SFG, we have studied the orientation and conformation of the liquid crystal molecule on clean and silane coated glass surfaces. On both surfaces, the biphenyl group is tilted by 70{degree} with the alkyl chain end pointing away from the surface. The shift in the C-H stretch frequencies in the coadsorbed system indicates a significant interaction between molecules. 9 refs., 3 figs.

  11. Resonant optical third-harmonic generation in few-layer black phosphorus

    NASA Astrophysics Data System (ADS)

    de Matos, Christiano J. S.; Rodrigues, Manuel J. L. F.; de Oliveira, Rafael E. P.; Peixoto, Hélder X. P.; Wu, Hsin-Yu; Wei, Ho Y.; Castro Neto, Antonio H.; Viana-Gomes, José C.

    Black phosphorus (BP), a layered monoatomic anisotropic crystal, has recently re-emerged due to demonstrations of its exfoliation down to few-layer thicknesses. It has been shown that BP remains a direct bandgap semiconductor from the bulk to the monolayer, which has triggered interest in its optoelectronic applications. However, optical characterization has been largely restricted to the linear regime, with nonlinear characterization limited to z-scan and saturable absorption measurements. In this work, we show optical third-harmonic generation measurements in bulk and few-layer BP. Results indicate a resonant increase in the generation efficiency of the latter, with signal intensities reaching values three orders of magnitude higher then those of graphene. The mechanisms leading to the resonant increase will be discussed. This work is supported by Fapesp (2012/50259-8 and 2015/11779-4), MackPesquisa, NRF-CRP (R-144-000-295-281), and NRF - Medium Sized Centre Programme.

  12. High harmonic generation in VUV via passive enhancement of near infrared femtosecond pulses

    NASA Astrophysics Data System (ADS)

    Wakui, Kentaro; Hayasaka, Kazuhiro; Ido, Tetsuya

    2011-10-01

    We generate a VUV frequency comb centered at 159 nm as the 5th harmonic of Ti:S femto-second pulses by a passive enhancement using an external cavity. Average power up to 1.5 uW is measured by a solar-blind phototube. Stable generation about 10 minutes is obtained by active locking of the Ti:S frequencies to the enhancement cavity. Frequency tunability of our Ti:S comb teeth is also verified, which enables us to continuously sweep its frequency with more than twice a free spectral range. Those features reported here are indispensable to precision spectroscopy of unexplored atomic transitions in the VUV region.

  13. Photoinduced second harmonic generation in partially crystallized BiB 3O 6 glass

    NASA Astrophysics Data System (ADS)

    Kityk, I. V.; Imiołek, W.; Majchrowski, A.; Michalski, E.

    2003-04-01

    Photoinduced second harmonic generation was found in BiB 3O 6 (BiBO) glass having different degree of crystallinity. We have revealed that an increasing degree of crystallinity of BiBO glass leads to increase of the output second-order optical susceptibility. We have used a pulsed 35 MW nitrogen laser ( λ=337 nm; τ=50 ps) as a source of photoinducing laser beam. Fundamental laser beam was generated by pulsed Nd:YAG laser ( λ=1.06 μm; time duration about 25 ps). Maximal value of the photoinduced second-order non-linear optical susceptibility d222 was equal to about 5 pm/V, what is substantially higher than in case of BiBO single crystals (˜ 3 pm/ V).

  14. High second harmonic generation signal from muscles and fascia pig's muscles using the two-photon laser scanning microscope.

    PubMed

    Reshak, A H

    2009-06-01

    I have provided update to our two photon laser scanning microscope by adding new technique which enables us to simultaneously measured the second harmonic generation signals in the forward and backward directions; in the meantime, one can measure the two photon excitations fluorescence if the materials produce fluorescence. In the present work, the fascia muscles, muscles of pig and pig's skin were used. I found that these materials produced high second harmonic generation signal in both directions. These measurements show that the second harmonic generation strongly depends on the state of the polarization of the laser light and the orientation of the dipole moment in the molecules that interact with the laser light. It is therefore advantageous to control the laser's state of polarization, to maximize second harmonic generation. The novelty of this work is to establish new multi-functional technique by combing three platforms of laser scanning microscopy - the fluorescence microscopy, harmonic generation microscopy and polarizing microscopy in which one can use the second harmonic imaging to investigate the true architecture of the sensitive samples and the samples which do not produce auto-fluorescence. Moreover investigation of the new sample needs to look at all details of the true architecture of the sample. Thereby the sample will be exposed to the laser radiation more than the well-known sample, and that will cause photo-bleaching and photo-damage. Since the second harmonic generation does not undergo from photo-bleaching and photo-damage it will be the promising technique for investigating the sensitive and new samples. Then one can move to acquire fluorescence images after good investigation of the true architecture of the sample by the SH imaging.

  15. Measurement of optical-beat frequency in a photoconductive terahertz-wave generator using microwave higher harmonics

    NASA Astrophysics Data System (ADS)

    Murasawa, Kengo; Sato, Koki; Hidaka, Takehiko

    2011-05-01

    A new method for measuring optical-beat frequencies in the terahertz (THz) region using microwave higher harmonics is presented. A microwave signal was applied to the antenna gap of a photoconductive (PC) device emitting a continuous electromagnetic wave at about 1 THz by the photomixing technique. The microwave higher harmonics with THz frequencies are generated in the PC device owing to the nonlinearity of the biased photoconductance, which is briefly described in this article. Thirteen nearly periodic peaks in the photocurrent were observed when the microwave was swept from 16 to 20 GHz at a power of -48 dBm. The nearly periodic peaks are generated by the homodyne detection of the optical beat with the microwave higher harmonics when the frequency of the harmonics coincides with the optical-beat frequency. Each peak frequency and its peak width were determined by fitting a Gaussian function, and the order of microwave harmonics was determined using a coarse (i.e., lower resolution) measurement of the optical-beat frequency. By applying the Kalman algorithm to the peak frequencies of the higher harmonics and their standard deviations, the optical-beat frequency near 1 THz was estimated to be 1029.81 GHz with the standard deviation of 0.82 GHz. The proposed method is applicable to a conventional THz-wave generator with a photomixer.

  16. Measurement of optical-beat frequency in a photoconductive terahertz-wave generator using microwave higher harmonics.

    PubMed

    Murasawa, Kengo; Sato, Koki; Hidaka, Takehiko

    2011-05-01

    A new method for measuring optical-beat frequencies in the terahertz (THz) region using microwave higher harmonics is presented. A microwave signal was applied to the antenna gap of a photoconductive (PC) device emitting a continuous electromagnetic wave at about 1 THz by the photomixing technique. The microwave higher harmonics with THz frequencies are generated in the PC device owing to the nonlinearity of the biased photoconductance, which is briefly described in this article. Thirteen nearly periodic peaks in the photocurrent were observed when the microwave was swept from 16 to 20 GHz at a power of -48 dBm. The nearly periodic peaks are generated by the homodyne detection of the optical beat with the microwave higher harmonics when the frequency of the harmonics coincides with the optical-beat frequency. Each peak frequency and its peak width were determined by fitting a Gaussian function, and the order of microwave harmonics was determined using a coarse (i.e., lower resolution) measurement of the optical-beat frequency. By applying the Kalman algorithm to the peak frequencies of the higher harmonics and their standard deviations, the optical-beat frequency near 1 THz was estimated to be 1029.81 GHz with the standard deviation of 0.82 GHz. The proposed method is applicable to a conventional THz-wave generator with a photomixer.

  17. Life Cycle Greenhouse Gas Emissions of Nuclear Electricity Generation: Systematic Review and Harmonization

    SciTech Connect

    Warner, E. S.; Heath, G. A.

    2012-04-01

    A systematic review and harmonization of life cycle assessment (LCA) literature of nuclear electricity generation technologies was performed to determine causes of and, where possible, reduce variability in estimates of life cycle greenhouse gas (GHG) emissions to clarify the state of knowledge and inform decision making. LCA literature indicates that life cycle GHG emissions from nuclear power are a fraction of traditional fossil sources, but the conditions and assumptions under which nuclear power are deployed can have a significant impact on the magnitude of life cycle GHG emissions relative to renewable technologies. Screening 274 references yielded 27 that reported 99 independent estimates of life cycle GHG emissions from light water reactors (LWRs). The published median, interquartile range (IQR), and range for the pool of LWR life cycle GHG emission estimates were 13, 23, and 220 grams of carbon dioxide equivalent per kilowatt-hour (g CO{sub 2}-eq/kWh), respectively. After harmonizing methods to use consistent gross system boundaries and values for several important system parameters, the same statistics were 12, 17, and 110 g CO{sub 2}-eq/kWh, respectively. Harmonization (especially of performance characteristics) clarifies the estimation of central tendency and variability. To explain the remaining variability, several additional, highly influential consequential factors were examined using other methods. These factors included the primary source energy mix, uranium ore grade, and the selected LCA method. For example, a scenario analysis of future global nuclear development examined the effects of a decreasing global uranium market-average ore grade on life cycle GHG emissions. Depending on conditions, median life cycle GHG emissions could be 9 to 110 g CO{sub 2}-eq/kWh by 2050.

  18. Mid-infrared ultrafast laser pulses induced third harmonic generation in nitrogen molecules on an excited state

    PubMed Central

    Xie, Hongqiang; Li, Guihua; Yao, Jinping; Chu, Wei; Li, Ziting; Zeng, Bin; Wang, Zhanshan; Cheng, Ya

    2015-01-01

    We report on generation of third harmonic from nitrogen molecules on the excited state with a weak driver laser pulse at a mid-infrared wavelength. The excited nitrogen molecules are generated using a circularly polarized intense femtosecond pulse which produces energetic electrons by photoionization to realize collisional excitation of nitrogen molecules. Furthermore, since the third harmonic is generated using a pump-probe scheme, it enables investigation of the excited-state dynamics of nitrogen molecules produced under different conditions. We also perform a comparative investigation in excited argon atoms, revealing different decay dynamics of the molecules and atoms from the excited states in femtosecond laser induced filaments. PMID:26522886

  19. Mid-infrared ultrafast laser pulses induced third harmonic generation in nitrogen molecules on an excited state.

    PubMed

    Xie, Hongqiang; Li, Guihua; Yao, Jinping; Chu, Wei; Li, Ziting; Zeng, Bin; Wang, Zhanshan; Cheng, Ya

    2015-11-02

    We report on generation of third harmonic from nitrogen molecules on the excited state with a weak driver laser pulse at a mid-infrared wavelength. The excited nitrogen molecules are generated using a circularly polarized intense femtosecond pulse which produces energetic electrons by photoionization to realize collisional excitation of nitrogen molecules. Furthermore, since the third harmonic is generated using a pump-probe scheme, it enables investigation of the excited-state dynamics of nitrogen molecules produced under different conditions. We also perform a comparative investigation in excited argon atoms, revealing different decay dynamics of the molecules and atoms from the excited states in femtosecond laser induced filaments.

  20. Revealing molecular structure and dynamics through high harmonic generation driven by mid-IR fields

    NASA Astrophysics Data System (ADS)

    Marangos, Jonathan

    2010-03-01

    High harmonic generation (HHG) from molecules has recently been shown to be a promising tool for measuring instantaneous molecular structure, sub-femtosecond domain structural rearrangements in molecules and even hole dynamics initiated by laser field ionisation. To fully exploit this promise it is essential that we can; (1) systematically decouple structural and dynamic effects so that both may simultaneously be determined in the measurement, (2) can extend the method of molecular HHG imaging to a wide range of molecules. Here we demonstrate important steps towards both these objectives. Up until now HHG imaging measurements have been restricted to drive laser wavelengths close to 800nm, due to the availability of CPA titanium sapphire lasers, which dictates the use of relatively high intensities (> 2.5 x 10^14 Wcm-2) if a harmonic spectrum spanning to ˜70 eV is to be observed which is required for extracting structural data from most small molecules. By using a mid-IR laser (at 1300 nm) we show that with an intensity ˜ 1 x 10^14 W cm-2 we can observe a wide molecular harmonic spectrum spanning to ˜ 70 eV even in molecules where ionization saturation would clamp the cut-off to much lower energies if an 800nm field were used. Thus we have been able to observe evidence for two-centre interference in two new molecules, N2O and C2H2 for the first time. Moreover we can use the ability to observe a broad harmonic spectrum over a large range of intensities to reveal the subtle interplay between structural and dynamic effects in CO2 and so provide a new window into hole dynamics. [4pt] In collaboration with R. Torres, Blackett Laboratory, Imperial College London; O. Smirnova, Max-Born-Institute, Berlin; T. Siegel and L. Brugnera, Blackett Laboratory, Imperial College London; I. Procino and Jonathan G. Underwood, Department of Physics and Astronomy, University College London; C. Altucci and R. Velotta, CNSIM and Dipartimento di Scienze Fisiche, Universita di Napoli