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Sample records for kondo resonance behaviors

  1. Lateral manipulation and interplay of local Kondo resonances in a two-impurity Kondo system

    SciTech Connect

    Ren, Jindong; Wu, Xu; Guo, Haiming Pan, Jinbo; Du, Shixuan; Gao, Hong-Jun; Luo, Hong-Gang

    2015-08-17

    The atomic-scale spatial relationship of a two-impurity Kondo system has been determined at varying lateral distance by scanning tunneling microscopy (STM) and spectroscopy. The localized spins of two cobalt magnetic adatoms that are placed on different electrodes of an STM form two individual Kondo singlet states, each showing quite different Kondo coupling, i.e., the tip-Kondo with low Kondo temperature and the sample-Kondo with high Kondo temperature. The differential conductance dI/dV spectra show the continuous changes of the resonance peak feature when approaching the Kondo tip laterally to the local sample-Kondo impurity on the surface. The result indicates a notable interplay between these two Kondo systems. We propose a convolution model based on the q factor of the sample-Kondo (q{sub s}) and tip-Kondo (q{sub t}) to interpret the change of various tunneling channels and the evolution of the experimental spectra.

  2. Spins of adsorbed molecules investigated by the detection of Kondo resonance

    NASA Astrophysics Data System (ADS)

    Komeda, Tadahiro

    2014-12-01

    Surface magnetism has been one of the platforms to explore the magnetism in low dimensions. It is also a key component for the development of quantum information processes, which utilizes the spin degree of freedom. The Kondo resonance is a phenomenon that is caused by an interaction between an isolated spin and conduction electrons. First observed in the 1930s as an anomalous increase in the low-temperature resistance of metals embedded with magnetic atoms, the Kondo physics mainly studied the effects of bulk magnetic impurities in the resistivity. In the last 15 years it has undergone a revival by a scanning tunneling microscope (STM) which enables the measurement of the Kondo resonance at surfaces using an atomic scale point contact. The detection of the Kondo resonance can be a powerful tool to explore surface magnetism. In this article, I review recent studies of the surface spin of adsorbed molecules by the detection of the Kondo resonance. Researches on metal phthalocyanine (MPc) and porphyrin molecules will be examined. In addition, the Kondo resonance for double-decker lanthanoide Pc molecules will be discussed. Some of the double-decker Pc molecules show single-molecule magnet (SMM) behavior, which attracts attention as a material for electronic devices. For both classes, the ligand plays a crucial role in determining the parameters of the Kondo resonance, such as the Kondo temperature and the change of the shape from peak to Fano-dip. In addition, the spin in delocalized molecular orbital forms the Kondo resonance, which shows significant differences from the Kondo resonance formed by the metal spins. Since molecular orbital can be tuned in a flexible manner by the design of the molecule, the Kondo resonance formed by delocalized molecular orbital might expand the knowledge of this field.

  3. Inelastic tunneling spectroscopy for magnetic atoms and the Kondo resonance.

    PubMed

    Goldberg, E C; Flores, F

    2013-06-05

    The interaction between a single magnetic atom and the metal environment (including a magnetic field) is analyzed by introducing an ionic Hamiltonian combined with an effective crystal-field term, and by using a Green-function equation of motion method. This approach describes the inelastic electron tunneling spectroscopy and the Kondo resonances as due to atomic spin fluctuations associated with electron co-tunneling processes between the leads and the atom. We analyze in the case of Fe on CuN the possible spin fluctuations between states with S = 2 and 3/2 or 5/2 and conclude that the experimentally found asymmetries in the conductance with respect to the applied bias, and its marked structures, are well explained by the 2↔3/2 spin fluctuations. The case of Co is also considered and shown to present, in contrast with Fe, a resonance at the Fermi energy corresponding to a Kondo temperature of 6 K.

  4. Lateral Fano resonances and Kondo effect in the strong coupling regime of a T -coupled quantum dot

    NASA Astrophysics Data System (ADS)

    Franco, R.; Figueira, M. S.; Anda, E. V.

    2006-05-01

    We study the electronic transport through a quantum wire (QW), modeled by a tight-binding linear chain, with a side-coupled quantum dot (QD). We obtain the conductance with a strong Fano antiresonance. The calculated density of states shows that this behavior is associated to a many-body renormalized QD resonant level Ef˜ at the edge of the conduction band (CB) strongly hybridized with the Van Hove singularity of the one-dimensional density of states of the lead. Different from the Fano antiresonances experimentally found when this system is at the Kondo regime, this phenomenon appears above the Kondo temperature. It is due to the quantum interference between the ballistic channel and a thermal activated channel created by the QD resonance at the vicinity of the bottom of the CB.

  5. Self-sustained oscillations in nanoelectromechanical systems induced by Kondo resonance

    NASA Astrophysics Data System (ADS)

    Song, Taegeun; Kiselev, Mikhail N.; Kikoin, Konstantin; Shekhter, Robert I.; Gorelik, Leonid Y.

    2014-03-01

    We investigate the instability and dynamical properties of nanoelectromechanical systems represented by a single-electron device containing movable quantum dots attached to a vibrating cantilever via asymmetric tunnel contacts. The Kondo resonance in electron tunneling between the source and shuttle facilitates self-sustained oscillations originating from the strong coupling of mechanical and electronic/spin degrees of freedom. We analyze a stability diagram for the two-channel Kondo shuttling regime due to limitations given by the electromotive force acting on a moving shuttle, and find that the saturation oscillation amplitude is associated with the retardation effect of the Kondo cloud. The results shed light on possible ways to experimentally realize the Kondo-cloud dynamical probe by using high mechanical dissipation tunability as well as supersensitive detection of mechanical displacement.

  6. Kondo resonance from p-wave hybridization in graphene.

    PubMed

    Jafari, S A; Tohyama, T

    2014-10-15

    The p-wave hybridization in graphene present a distinct class of Kondo problem in pseudogap Fermi systems with bath density of states (DOS) ρ₀(ε) ∝ |ε|. The peculiar geometry of substitutional and hollow-site ad-atoms, and effectively the vacancies allow for a p-wave form of momentum dependence in the hybridization of the associated local orbital with the Dirac fermions of the graphene host which results in a different picture than the s-wave momentum independent hybridization. For the p-wave hybridization function, away from the Dirac point we find closed-form formulae for the Kondo temperature TK which in contrast to the s-wave case is non-zero for any value of hybridization strength V of the single impurity Anderson model (SIAM). At the Dirac point where the DOS vanishes, we find a conceivably small value of Vmin above which the Kondo screening takes place even in the presence of particle-hole symmetry. We also show that the non-Lorentzian line shape of the local spectrum arising from anomalous hybridization function leads to much larger TK in vacant graphene compared to a metallic host with similar bandwidth and SIAM parameters.

  7. Sub-molecular modulation of a 4f driven Kondo resonance by surface-induced asymmetry

    PubMed Central

    Warner, Ben; El Hallak, Fadi; Atodiresei, Nicolae; Seibt, Philipp; Prüser, Henning; Caciuc, Vasile; Waters, Michael; Fisher, Andrew J.; Blügel, Stefan; van Slageren, Joris; Hirjibehedin, Cyrus F.

    2016-01-01

    Coupling between a magnetic impurity and an external bath can give rise to many-body quantum phenomena, including Kondo and Hund's impurity states in metals, and Yu-Shiba-Rusinov states in superconductors. While advances have been made in probing the magnetic properties of d-shell impurities on surfaces, the confinement of f orbitals makes them difficult to access directly. Here we show that a 4f driven Kondo resonance can be modulated spatially by asymmetric coupling between a metallic surface and a molecule containing a 4f-like moment. Strong hybridization of dysprosium double-decker phthalocyanine with Cu(001) induces Kondo screening of the central magnetic moment. Misalignment between the symmetry axes of the molecule and the surface induces asymmetry in the molecule's electronic structure, spatially mediating electronic access to the magnetic moment through the Kondo resonance. This work demonstrates the important role that molecular ligands have in mediating electronic and magnetic coupling and in accessing many-body quantum states. PMID:27666413

  8. Blocking transport resonances via Kondo many-body entanglement in quantum dots

    PubMed Central

    Niklas, Michael; Smirnov, Sergey; Mantelli, Davide; Margańska, Magdalena; Nguyen, Ngoc-Viet; Wernsdorfer, Wolfgang; Cleuziou, Jean-Pierre; Grifoni, Milena

    2016-01-01

    Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we show another side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic co-tunnelling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global SU(2) ⊗ SU(2) symmetry of a nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin. PMID:27526870

  9. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: Kondo Resonance Splitting in a Quantum Dot with Perpendicular Magnetic Fields

    NASA Astrophysics Data System (ADS)

    Peng, Ju; Yu, Hua-Ling; Wang, Xia-Ling; Chen, Zhi-Gao

    2009-12-01

    Using the nonequilibrium Green's function technique, we investigate the Kondo effect in the quantum dot with perpendicular magnetic fields, in which one is the Zeeman splitting lies in the z-direction and the other is the spin flip points at the x-direction. It is found whatever one or two magnetic fields are applied, the local density of states (LDOS) will split into two peaks. The positions of two Kondo resonance peaks are determined by Zeeman energy Δ when J = 0, and by when J ≠ 0.

  10. Kondo Resonance in a Mesoscopic Ring Coupled to a Quantum Dot: Exact Results for the Aharonov-Bohm-Casher Effects

    SciTech Connect

    Eckle, H.-P.; Johannesson, H.; Stafford, C. A.

    2001-07-02

    We study the persistent currents induced by both the Aharonov-Bohm and Aharonov-Casher effects in a one-dimensional mesoscopic ring coupled to a sidebranch quantum dot at Kondo resonance. For privileged values of the Aharonov-Bohm-Casher fluxes, the problem can be mapped onto an integrable model, exactly solvable by a Bethe ansatz. In the case of a pure magnetic Aharonov-Bohm flux, we find that the presence of the quantum dot has no effect on the persistent current. In contrast, the Kondo resonance interferes with the spin-dependent Aharonov-Casher effect to induce a current which, in the strong-coupling limit, is independent of the number of electrons in the ring.

  11. Kondo resonance in a mesoscopic ring coupled to a quantum dot: exact results for the Aharonov-Bohm-Casher effects.

    PubMed

    Eckle, H P; Johannesson, H; Stafford, C A

    2001-07-02

    We study the persistent currents induced by both the Aharonov-Bohm and Aharonov-Casher effects in a one-dimensional mesoscopic ring coupled to a sidebranch quantum dot at Kondo resonance. For privileged values of the Aharonov-Bohm-Casher fluxes, the problem can be mapped onto an integrable model, exactly solvable by a Bethe ansatz. In the case of a pure magnetic Aharonov-Bohm flux, we find that the presence of the quantum dot has no effect on the persistent current. In contrast, the Kondo resonance interferes with the spin-dependent Aharonov-Casher effect to induce a current which, in the strong-coupling limit, is independent of the number of electrons in the ring.

  12. Spin Relaxation in Kondo Lattice Systems with Anisotropic Kondo Interaction

    NASA Astrophysics Data System (ADS)

    Belov, S. I.; Kutuzov, A. S.

    2016-12-01

    We study the influence of the Kondo effect on the spin relaxation in systems with anisotropic Kondo interaction at temperatures both high and low as compared with the static magnetic field. In the absence of the Kondo effect, the electron spin resonance linewidth is not narrowed in the whole temperature range due to the high anisotropy of the Kondo interaction. The Kondo effect leads to the universal energy scale, which regulates the temperature and magnetic field dependence of different kinetic coefficients and results in a mutual cancelation of their singular parts in a collective spin mode.

  13. NMR evidence of anisotropic Kondo liquid behavior in CeIrIn5

    NASA Astrophysics Data System (ADS)

    Shockley, A. C.; Shirer, K. R.; Crocker, J.; Dioguardi, A. P.; Lin, C. H.; Nisson, D. M.; apRoberts-Warren, N.; Klavins, P.; Curro, N. J.

    2015-08-01

    We report detailed Knight-shift measurements of the two indium sites in the heavy-fermion compound CeIrIn5 as a function of temperature and field orientation. We find that the Knight-shift anomaly is orientation dependent, with a crossover temperature T* that varies by 50% as the field is rotated from (001) to (100). This result suggests that the hybridization between the Ce 4 f states and the itinerant conduction electrons is anisotropic, a result that reflects its collective origin, and may lead to anisotropic Kondo liquid behavior and unconventional superconductivity.

  14. Corrected Kondo temperature beyond the conventional Kondo scaling limit.

    PubMed

    Li, ZhenHua; Wei, JianHua; Zheng, Xiao; Yan, YiJing; Luo, Hong-Gang

    2017-02-20

    In the Kondo systems such as the magnetic impurity screened by the conduction electrons in a metal host, as well as the quantum dots connected by the leads, the low energy behaviors have universal dependence on the [Formula: see text] or [Formula: see text], where [Formula: see text] is the conventional Kondo temperature. However, it was shown that this scaling behavior is only valid at low-energy; this is called the Kondo scaling limit. Here we explore the extention of the scaling parameter range by introducing the corrected Kondo temperature T K, which may depend on the temperature and bias, as well as the other external parameters. We define the corrected Kondo temperature by scaling the local density of states near the Fermi level, obtained by accurate hierarchy of equations of motion approach at finite temperature and finite bias, and thus obtain a phenomenological expression of the corrected Kondo temperature. By using the corrected Kondo temperature as a characteristic energy scale, the conductance of the quantum dot can be well scaled in a wide parameter range, even two orders beyond the conventional scaling parameter range. Our work indicates that the Kondo scaling, although dominated by the conventional Kondo temperature in the low-energy of the Kondo system, could be extended to a higher energy regime, which is useful for analyzing the physics of the Kondo transport in non-equilibrium or high temperature cases.

  15. Kondo behavior and conductance through 3d impurities in gold chains doped with oxygen

    NASA Astrophysics Data System (ADS)

    Barral, M. A.; Di Napoli, S.; Blesio, G.; Roura-Bas, P.; Camjayi, A.; Manuel, L. O.; Aligia, A. A.

    2017-03-01

    Combining ab initio calculations and effective models derived from them, we discuss the electronic structure of oxygen doped gold chains when one Au atom is replaced by any transition-metal atom of the 3d series. The effect of O doping is to bring extended Au 5dxz and 5dyz states to the Fermi level, which together with the Au states of zero angular momentum projection leads to three possible channels for the screening of the magnetism of the impurity. For most 3d impurities the expected physics is similar to that of the underscreened Kondo model, with singular Fermi liquid behavior. For Fe and Co under a tetragonal crystal field introduced by leads, the system might display a non-Fermi liquid behavior. Ni and Cu impurities are described by a S = 1 two channel Kondo model and an SU(4) impurity Anderson model in the intermediate valence regime, respectively. In both cases, the system is a Fermi liquid, but the conductance shows some observable differences with the ordinary SU(2) Anderson model.

  16. Heavy fermion and Kondo lattice behavior in the itinerant ferromagnet CeCrGe3.

    PubMed

    Das, Debarchan; Gruner, T; Pfau, H; Paramanik, U B; Burkhardt, U; Geibel, C; Hossain, Z

    2014-03-12

    Physical properties of polycrystalline CeCrGe3 and LaCrGe3 have been investigated by x-ray absorption spectroscopy, magnetic susceptibility χ(T), isothermal magnetization M(H), electrical resistivity ρ(T), specific heat C(T) and thermoelectric power S(T) measurements. These compounds are found to crystallize in the hexagonal perovskite structure (space group P63/mmc), as previously reported. The ρ(T), χ(T) and C(T) data confirm the bulk ferromagnetic ordering of itinerant Cr moments in LaCrGe3 and CeCrGe3 with TC = 90 K and 70 K respectively. In addition, a weak anomaly is also observed near 3 K in the C(T) data of CeCrGe3. The T dependences of ρ and finite values of Sommerfeld coefficient γ obtained from the specific heat measurements confirm that both the compounds are of metallic character. Further, the T dependence of ρ of CeCrGe3 reflects a Kondo lattice behavior. An enhanced γ of 130 mJ mol(-1) K(-2) together with the Kondo lattice behavior inferred from the ρ(T) establish CeCrGe3 as a moderate heavy fermion compound with a quasi-particle mass renormalization factor of ∼45.

  17. Theory of Fano Resonances in Graphene: The Kondo effect probed by STM

    SciTech Connect

    Wehling, T.O.

    2010-06-02

    We consider the theory of Kondo effect and Fano factor energy dependence for magnetic impurity (Co) on graphene. We have performed a first principles calculation and find that the two dimensional E{sub 1} representation made of d{sub xz}, d{sub yz} orbitals is likely to be responsible for the hybridization and ultimately Kondo screening for cobalt on graphene. There are few high symmetry sites where magnetic impurity atom can be adsorbed. For the case of Co atom in the middle of hexagon of carbon lattice we find anomalously large Fano q-factor, q {approx} 80 and strongly suppressed coupling to conduction band. This anomaly is a striking example of quantum mechanical interference related to the Berry phase inherent to graphene band structure.

  18. Kondo lattice heavy fermion behavior in CeRh2Ga2.

    PubMed

    Anand, V K; Adroja, D T; Bhattacharyya, A; Klemke, B; Lake, B

    2017-04-05

    The physical properties of an intermetallic compound CeRh2Ga2 have been investigated by magnetic susceptibility [Formula: see text], isothermal magnetization M(H), heat capacity [Formula: see text], electrical resistivity [Formula: see text], thermal conductivity [Formula: see text] and thermopower S(T) measurements. CeRh2Ga2 is found to crystallize with CaBe2Ge2-type primitive tetragonal structure (space group P4/nmm). No evidence of long range magnetic order is seen down to 1.8 K. The [Formula: see text] data show paramagnetic behavior with an effective moment [Formula: see text]/Ce indicating Ce(3+) valence state of Ce ions. The [Formula: see text] data exhibit Kondo lattice behavior with a metallic ground state. The low-T [Formula: see text] data yield an enhanced Sommerfeld coefficient [Formula: see text] mJ/mol K(2) characterizing CeRh2Ga2 as a moderate heavy fermion system. The high-T [Formula: see text] and [Formula: see text] show an anomaly near 255 K, reflecting a phase transition. The [Formula: see text] suggests phonon dominated thermal transport with considerably higher values of Lorenz number L(T) compared to the theoretical Sommerfeld value L 0.

  19. Kondo lattice heavy fermion behavior in CeRh2Ga2

    NASA Astrophysics Data System (ADS)

    Anand, V. K.; Adroja, D. T.; Bhattacharyya, A.; Klemke, B.; Lake, B.

    2017-04-01

    The physical properties of an intermetallic compound CeRh2Ga2 have been investigated by magnetic susceptibility χ (T) , isothermal magnetization M(H), heat capacity {{C}\\text{p}}(T) , electrical resistivity ρ (T) , thermal conductivity κ (T) and thermopower S(T) measurements. CeRh2Ga2 is found to crystallize with CaBe2Ge2-type primitive tetragonal structure (space group P4/nmm). No evidence of long range magnetic order is seen down to 1.8 K. The χ (T) data show paramagnetic behavior with an effective moment {μ\\text{eff}}≈ 2.5~{μ\\text{B}} /Ce indicating Ce3+ valence state of Ce ions. The ρ (T) data exhibit Kondo lattice behavior with a metallic ground state. The low-T {{C}\\text{p}}(T) data yield an enhanced Sommerfeld coefficient γ =130(2) mJ/mol K2 characterizing CeRh2Ga2 as a moderate heavy fermion system. The high-T {{C}\\text{p}}(T) and ρ (T) show an anomaly near 255 K, reflecting a phase transition. The κ (T) suggests phonon dominated thermal transport with considerably higher values of Lorenz number L(T) compared to the theoretical Sommerfeld value L 0.

  20. Spatially dependent Kondo effect in Quantum Corrals

    NASA Astrophysics Data System (ADS)

    Rossi, Enrico; Morr, Dirk K.

    2007-03-01

    We study the Kondo screening of a single magnetic impurity placed inside a quantum corral consisting of non-magnetic impurities on the surface of a metallic host system. We show that the spatial structure of the corral's eigenmodes leads to a spatially dependent Kondo effect whose signatures are experimentally measurable spatial variations of the Kondo temperature, TK, and of the critical Kondo coupling, Jcr. Moreover we find that the screening of the magnetic impurity is accompanied by the formation of multiple Kondo resonances with characteristic spatial patterns that provide further experimental signatures of the spatially dependent Kondo effect. Our results demonstrate that quantum corrals provide new possibilities to manipulate and explore the Kondo effect.

  1. Complex magnetic behavior in the novel Kondo lattice compound CeRhSn₃.

    PubMed

    Anand, V K; Adroja, D T; Hillier, A D; Kockelmann, W; Fraile, A; Strydom, A M

    2011-07-13

    We report the magnetic and transport properties of a new ternary intermetallic compound, CeRhSn₃, using magnetic susceptibility, magnetization, specific heat, electrical resistivity, muon-spin relaxation (μSR) and neutron diffraction investigations. The dc magnetic susceptibility data reveal two magnetic phase transitions at 0.9 and 4 K. The overall behavior of dc susceptibility and magnetization indicates a ferrimagnetic-type phase transition near 4 K. The specific heat data also exhibit sharp λ-type anomalies at 1 and 4 K. The behavior of the specific heat anomaly under the application of a magnetic field suggests that the 1 K transition is probably related to a transition from a ferri- to a ferromagnetic state. The low temperature specific heat exhibits an enhanced Sommerfeld coefficient γ (~100 mJ mol⁻¹ K⁻²) due to the formation of a moderate heavy fermion state. The resistivity of CeRhSn₃ demonstrates an interplay between the RKKY and Kondo interactions which is further modified by the presence of the crystal electric field. Interestingly, the resistivity of the nonmagnetic reference compound, LaRhSn₃, is found to increase with decreasing temperature. Further, the onset of long-range magnetic order below 1 K is confirmed from our μSR study on CeRhSn₃. However, the 4 K transition is not detected in the μSR and low temperature neutron diffraction data. Analysis of the dc magnetic susceptibility data within the framework of a two-sublattice model of ferrimagnetism supports the ferrimagnetic-type transition at 4 K in CeRhSn₃. We have observed an unusual frequency dependence of the peak near 4 K in the ac susceptibility, which shows that the transition temperature shifts toward the lower temperature side with increasing frequency.

  2. The effect of Ce dilution on the ferromagnetic ordering and Kondo behavior of CeRuPO

    NASA Astrophysics Data System (ADS)

    Noorafshan, M.; Nourbakhsh, Z.

    2017-03-01

    The structural, electronic and magnetic properties and Kondo behavior of Ce1-xLax RuPO (x=0, 0.25, 0.5, 0.75 and 1) alloys are investigated using density functional theory by utilizing Wien2k package. The exchange-correlation potential is treated with the generalized gradient approximation (GGA). Moreover, the GGA+U approach (where U is the Hubbard correlation term) is employed to treat the f-electrons properly. We also present a comparative study between the electronic structure and magnetic properties of these alloys within GGA and GGA+U approaches. The calculated lattice parameters and bulk moduli of these alloys as a function of x are in the best agreement with Vegard's linear rule. The total and partial electron density of states and linear coefficient of electronic specific heat of these alloy within GGA and GGA+U are investigated and compared. The effect of La substitution on the Kondo behavior of CeRuPO compound is investigated.

  3. Quantum Critical Behavior of the Bose-Fermi Kondo Model with Ising Anisotropy

    NASA Astrophysics Data System (ADS)

    Park, Tae-Ho

    2005-03-01

    The existence of a continous quantum phase transition of the Bose-Fermi Kondo Model (BFKM) with a self-consistently determined bosonic bath has been demonstrated within the Extended Dynamical Mean Field Approach to the anisotropic Kondo lattice model and φ/T-scaling near the quantum critical point(QCP)was found[1,2]. We study the quantum critical properties of the anisotropic BFKM with specified bath spectral function, where the spectrum of the bosonic bath vanishes in a power-law fashion with exponent γ for small frequencies. Motivated by very recent results that the quantum to classical mapping for a related class of models fails[3,4]. We determine the critical local susceptibility using both the classical and quantum Monte Carlo approaches of Ref.5. Our results cover several values of γ below and above the upper critical dimension of the classical model for temperatures down to 1% of the bare Kondo scale. [1]D. Grempel and Q. Si, Phys. Rev. Lett. 91, 026402 (2003). [2]J.Zhu, D. Grempel, and Q. Si, Phys. Rev. Lett. 91, 156404 (2003). [3]L. Zhu, S. Kirchner, Q. Si nad A. Georges, Phys. Rev. Lett. in press (cond-mat/0406293). [4]M. Vojta, N. Tong, and R. Bulla, cond-mat/0410132. [5]D. Grempel and M. Rozenberg, Phys. Rev. B 60, 4702 (1999).

  4. Enhanced superconductivity, Kondo behavior, and negative-curvature resistivity of oxygen-irradiated thin films of aluminium

    NASA Astrophysics Data System (ADS)

    Sinnecker, E. H. C. P.; Sant'Anna, M. M.; ElMassalami, M.

    2017-02-01

    We followed the evolution of the normal and superconducting properties of Al thin films after each session of various successive oxygen irradiations at ambient temperature. Such irradiated films, similar to the granular ones, exhibit enhanced superconductivity, Kondo behavior, and negative-curvature resistivity. Two distinct roles of oxygen are identified: as a damage-causing projectile and as an implanted oxidizing agent. The former gives rise to the processes involved in the conventional recovery stages. The latter, considered within the context of the Cabrera-Mott model, gives rise to a multistep process which involves charges transfer and creation of stabilized vacancies and charged defects. Based on the outcome of this multistep process, we consider (i) the negative-curvature resistivity as a manifestation of a thermally assisted liberation of trapped electric charges, (ii) the Kondo contribution as a spin-flip scattering from paramagnetic, color-center-type defects, and (iii) the enhancement of Tc as being due to a lattice softening facilitated by the stabilized defects and vacancies. The similarity in the phase diagrams of granular and irradiated films as well as the aging effects are discussed along the same line of reasoning.

  5. Kondo physics in the single-electron transistor with ac driving

    NASA Astrophysics Data System (ADS)

    Nordlander, Peter; Wingreen, Ned S.; Meir, Yigal; Langreth, David C.

    2000-01-01

    Using a time-dependent Anderson Hamiltonian, a quantum dot with an ac voltage applied to a nearby gate is investigated. A rich dependence of the linear response conductance on the external frequency and driving amplitude is demonstrated. At low frequencies a sufficiently strong ac potential produces sidebands of the Kondo peak in the spectral density of the dot, and a slow, roughly logarithmic decrease in conductance over several decades of frequency. At intermediate frequencies, the conductance of the dot displays an oscillatory behavior due to the appearance of Kondo resonances of the satellites of the dot level. At high frequencies, the conductance of the dot can vary rapidly due to the interplay between photon-assisted tunneling and the Kondo resonance.

  6. The Kondo tip decorated by the Co atom

    NASA Astrophysics Data System (ADS)

    Feng, Wei; Liu, Qin; Lai, Xinchun; Zhao, Aidi

    2016-11-01

    The Kondo effect of single Co adatoms on Ru(0001) is detected with two different kinds of co-decorated tip (Kondo tip) by using low temperature scanning tunneling microscopy and scanning tunneling spectroscopy. We call the relatively separated two magnetic impurities in the tunneling region ‘two Kondo system’ to distinguish it from the ‘two-impurity Kondo system’. We find that the artificially constructed Kondo tips can be generally categorized into two types of Kondo resonances, which have distinct Fano line shapes with quantum interference factor |q| ≫ 1 and |q| ∼ 1, respectively. The tunneling spectra of six constructed two Kondo systems can be well fitted by summing the two Fano resonances of the two subsystems and a linear background. More interestingly, by extracting the amplitudes of the two Fano resonances in the spectra, we find that the electron transmission of such a two Kondo system in the tunneling region is dominated by the quantum interference of the Kondo tip, which is directly related to the geometric configuration of the adsorbed Kondo atom on the tip.

  7. Kondo lattice and antiferromagnetic behavior in quaternary CeTAl4Si2 (T = Rh, Ir) single crystals

    DOE PAGES

    Maurya, Arvind; Kulkarni, Ruta; Thamizhavel, Arumugam; ...

    2016-02-26

    Here, we have explored in detail the anisotropic magnetic properties of CeRhAl4Si2 and CeIrAl4Si2, which undergo two antiferromagnetic transitions, at TN1 = 12.6 and 15.5 K, followed by a second transition at TN2 = 9.4 and 13.8 K, respectively, with the [001]-axis as the relatively easy axis of magnetization. The electrical resistivity at ambient and applied pressure provides evidence of Kondo interaction in both compounds, further supported by a reduced value of the entropy associated with the magnetic ordering. The Sommerfeld coefficient γ is inferred to be 195.6 and 49.4 mJ/(mol K2) for CeRhAl4Si2 and CeIrAl4Si2, respectively, classifying these materialsmore » as moderate heavy-fermion compounds. The crystal electric field energy levels are derived from the peak seen in the Schottky heat capacity. Furthermore, we have also performed electronic structure calculations by using the local spin density approximation + U [LSDA+U] approach, which provide physical insights on the observed magnetic behavior of these two compounds.« less

  8. Nonlinear behavior of Helmholtz resonators

    NASA Astrophysics Data System (ADS)

    Hersh, A. S.

    1990-10-01

    A semi-empirical fluid mechanical model has been derived to predict the nonlinear acoustic behavior of thin-walled, single-orifice Helmholtz resonators. The model assumed that the sound particle velocity field approaches the resonator in a spherically symmetric manner. The incident and cavity sound pressure fields are connected in terms of an orifice discharge coefficient and an end correction parameter whose values are determined empirically. The accuracy of the model was verified by comparing predicted with measured impedance over a wide range of sound amplitudes and frequencies for two different resonator geometries and with measurements conducted by Ingard and Ising.

  9. GW approach to Anderson model in and out of equilibrium : scaling properties in the Kondo regime.

    SciTech Connect

    Spataru, Dan Catalin

    2010-03-01

    The low-energy properties of the Anderson model for a single impurity coupled to two leads are studied using the GW approximation. We find that quantities such as the spectral function at zero temperature, the linear-response conductance as function of temperature or the differential conductance as function of bias voltage exhibit universal scaling behavior in the Kondo regime. We show how the form of the GW scaling functions relates to the form of the scaling functions obtained from the exact solution at equilibrium. We also compare the energy scale that goes inside the GW scaling functions with the exact Kondo temperature, for a broad range of the Coulomb interaction strength in the asymptotic regime. This analysis allows to clarify a presently suspended question in the literature, namely whether or not the GW solution captures the Kondo resonance.

  10. Transport signatures of Kondo physics and quantum criticality in graphene with magnetic impurities

    NASA Astrophysics Data System (ADS)

    Ruiz-Tijerina, David A.; Dias da Silva, Luis G. G. V.

    2017-03-01

    Localized magnetic moments have been predicted to develop in graphene samples with vacancies or adsorbates. The interplay between such magnetic impurities and graphene's Dirac quasiparticles leads to remarkable many-body phenomena, which have, so far, proved elusive to experimental efforts. In this article we study the thermodynamic, spectral, and transport signatures of quantum criticality and Kondo physics of a dilute ensemble of atomic impurities in graphene. We consider vacancies and adatoms that either break or preserve graphene's C3 v and inversion symmetries. In a neutral graphene sample, all cases display symmetry-dependent quantum criticality, leading to enhanced impurity scattering for asymmetric impurities, in a manner analogous to bound-state formation by nonmagnetic resonant scatterers. Kondo correlations emerge only in the presence of a back gate, with estimated Kondo temperatures well within the experimentally accessible domain for all impurity types. For symmetry-breaking impurities at charge neutrality, quantum criticality is signaled by T-2 resistivity scaling, leading to full insulating behavior at low temperatures, while low-temperature resistivity plateaus appear both in the noncritical and Kondo regimes. By contrast, the resistivity contribution from symmetric vacancies and hollow-site adsorbates vanishes at charge neutrality and for arbitrary back-gate voltages, respectively. This implies that local probing methods are required for the detection of both Kondo and quantum critical signatures in these symmetry-preserving cases.

  11. Spin versus charge noise from Kondo traps

    NASA Astrophysics Data System (ADS)

    da Silva, Luis G. G. V. Dias; de Sousa, Rogério

    2015-08-01

    Magnetic and charge noise have a common microscopic origin in solid-state devices, as described by a universal electron trap model. In spite of this common origin, magnetic (spin) and charge noise spectral densities display remarkably different behaviors when many-particle correlations are taken into account, leading to the emergence of the Kondo effect. We derive exact frequency sum rules for trap noise and perform numerical renormalization-group calculations to show that while spin noise is a universal function of the Kondo temperature, charge noise remains well described by single-particle theory even when the trap is deep in the Kondo regime. We obtain simple analytical expressions for charge and spin noise that account for Kondo screening in all frequency and temperature regimes, enabling the study of the impact of disorder and the emergence of magnetic 1 /f noise from Kondo traps. We conclude that the difference between charge and spin noise survives even in the presence of disorder, showing that noise can be more manageable in devices that are sensitive to magnetic (rather than charge) fluctuations and that the signature of the Kondo effect can be observed in spin noise spectroscopy experiments.

  12. Fano-Kondo and the Kondo box regimes crossover in a quantum dot coupled to a quantum box.

    PubMed

    Apel, Victor M; Orellana, Pedro A; Pacheco, Monica; Anda, Enrique V

    2013-12-18

    In this work, we study the Kondo effect of a quantum dot (QD) connected to leads and to a discrete set of one-particle states provided by a quantum box represented by a quantum ring (QR) pierced by a magnetic flux side attached to the QD. The interplay between the bulk Kondo effect and the so-called Kondo box regime is studied. In this system the QR energies can be continuously modified by the application of the magnetic field. The crossover between these two regimes is analyzed by changing the connection of the QD to the QR from the weak to the strong coupling regime. In the weak coupling regime, the differential conductance develops a sequence of Fano-Kondo anti-resonances due to destructive interference between the discrete quantum ring levels and the conducting Kondo channel provided by the leads. In the strong coupling regime the differential conductance has very sharp resonances when one of the Kondo discrete sub-levels characterizing the Kondo box is tuned by the applied potential. The conductance, the current fluctuations and the Fano coefficient result as being the relevant physical magnitudes to be analyzed to reveal the physical properties of these two Kondo regimes and the crossover region between them. The results were obtained by using the slave boson mean field theory (SBMFT).

  13. Photoinduced Kondo effect in CeZn3P3

    NASA Astrophysics Data System (ADS)

    Kitagawa, J.; Kitajima, D.; Shimokawa, K.; Takaki, H.

    2016-01-01

    The Kondo effect, which originates from the screening of a localized magnetic moment by a spin-spin interaction, is widely observed in nonartificial magnetic materials, artificial quantum dots, and carbon nanotubes. In devices based on quantum dots or carbon nanotubes that target quantum information applications, the Kondo effect can be tuned by a gate voltage, a magnetic field, or light. However, the manipulation of the Kondo effect in nonartificial materials has not been thoroughly studied; in particular, the artificial creation of the Kondo effect remains unexplored. Per this subject study, however, a route for the optical creation of the Kondo effect in the nonartificial material p -type semiconductor CeZn3P3 is presented. The Kondo effect emerges under visible-light illumination of the material by a continuous-wave laser diode and is ultimately revealed by photoinduced electrical resistivity, which clearly exhibits a logarithmic temperature dependency. By contrast, a La-based compound (LaZn3P3 ) displays only normal metallic behavior under similar illumination. The photoinduced Kondo effect, which occurs at higher temperatures when compared with the Kondo effect in artificial systems, provides a potential range of operation for not only quantum information/computation devices but also for operation of magneto-optic devices, thereby expanding the range of device applications based on the Kondo effect.

  14. Kondo peak splitting and Kondo dip in single molecular magnet junctions

    NASA Astrophysics Data System (ADS)

    Niu, Pengbin; Shi, Yunlong; Sun, Zhu; Nie, Yi-Hang; Luo, Hong-Gang

    2016-01-01

    Many factors containing bias, spin-orbit coupling, magnetic fields applied, and so on can strongly influence the Kondo effect, and one of the consequences is Kondo peak splitting (KPS). It is natural that KPS should also appear when another spin degree of freedom is involved. In this work we study the KPS effects of single molecular magnets (SMM) coupled with two metallic leads in low-temperature regime. It is found that the Kondo transport properties are strongly influenced by the exchange coupling and anisotropy of the magnetic core. By employing Green's function method in Hubbard operator representation, we give an analytical expression for local retarded Green's function of SMM and discussed its low-temperature transport properties. We find that the anisotropy term behaves as a magnetic field and the splitting behavior of exchange coupling is quite similar to the spin-orbit coupling. These splitting behaviors are explained by introducing inter-level or intra-level transitions, which account for the seven-peak splitting structure. Moreover, we find a Kondo dip at Fermi level under proper parameters. These Kondo peak splitting behaviors in SMM deepen our understanding to Kondo physics and should be observed in the future experiments.

  15. Manipulating Kondo temperature via single molecule switching.

    PubMed

    Iancu, Violeta; Deshpande, Aparna; Hla, Saw-Wai

    2006-04-01

    Two conformations of isolated single TBrPP-Co molecules on a Cu(111) surface are switched by applying +2.2 V voltage pulses from a scanning tunneling microscope tip at 4.6 K. The TBrPP-Co has a spin-active cobalt atom caged at its center, and the interaction between the spin of this cobalt atom and free electrons from the Cu(111) substrate can cause a Kondo resonance. Tunneling spectroscopy data reveal that switching from the saddle to a planar molecular conformation enhances spin-electron coupling, which increases the associated Kondo temperature from 130 to 170 K. This result demonstrates that the Kondo temperature can be manipulated just by changing molecular conformation without altering chemical composition of the molecule.

  16. Application of the underscreened Kondo lattice model to neptunium compounds

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simoes, Acirete S.; Iglesias, J. R.; Lacroix, C.; Coqublin, B.

    2012-12-01

    The coexistence of Kondo effect and ferromagnetic order has been observed in many uranium and neptunium compounds such as UTe or Np2PdGa3. This coexistence can be described within the underscreened Anderson lattice model with two f-electrons and S = 1 spins on each site. After performing the Schrieffer-Wolff transformation on this model, we have obtained an effective Hamiltonian with a f-band term in addition to the Kondo interaction for S = 1 spins. The results indicate a coexistence of Kondo effect and ferromagnetic order, with different relative values of the Kondo TK and Curie TC temperatures. We emphasize here especially the case TK < TC where there is a Kondo behavior below TC and a clear decrease of the magnetization below TK. Such a behavior has been observed in the magnetization curves of NpNiSi2 at low temperatures.

  17. From Kondo lattices to Kondo superlattices

    NASA Astrophysics Data System (ADS)

    Shimozawa, Masaaki; Goh, Swee K.; Shibauchi, Takasada; Matsuda, Yuji

    2016-07-01

    The realization of new classes of ground states in strongly correlated electron systems continues to be a major issue in condensed matter physics. Heavy fermion materials, whose electronic structure is essentially three-dimensional, are one of the most suitable systems for obtaining novel electronic states because of their intriguing properties associated with many-body effects. Recently, a state-of-the-art molecular beam epitaxy technique was developed to reduce the dimensionality of heavy electron systems by fabricating artificial superlattices that include heavy fermion compounds; this approach can produce a new type of electronic state in two-dimensional (2D) heavy fermion systems. In artificial superlattices of the antiferromagnetic heavy fermion compound CeIn3 and the conventional metal LaIn3, the magnetic order is suppressed by a reduction in the thickness of the CeIn3 layers. In addition, the 2D confinement of heavy fermions leads to enhancement of the effective electron mass and deviation from the standard Fermi liquid electronic properties, which are both associated with the dimensional tuning of quantum criticality. In the superconducting superlattices of the heavy fermion superconductor CeCoIn5 and nonmagnetic metal YbCoIn5, signatures of superconductivity are observed even at the thickness of one unit-cell layer of CeCoIn5. The most remarkable feature of this 2D heavy fermion superconductor is that the thickness reduction of the CeCoIn5 layers changes the temperature and angular dependencies of the upper critical field significantly. This result is attributed to a substantial suppression of the Pauli pair-breaking effect through the local inversion symmetry breaking at the interfaces of CeCoIn5 block layers. The importance of the inversion symmetry breaking in this system has also been supported by site-selective nuclear magnetic resonance spectroscopy, which can resolve spectroscopic information from each layer separately, even within the same CeCoIn5

  18. Interacting electrons and quenched randomness: From the mesoscopic Kondo problem to the depeleted Kondo lattice

    NASA Astrophysics Data System (ADS)

    Kaul, Ribhu

    The physics of strong electron-electron interactions in quantum many body physics is an exciting subject. An understanding of these effects is crucial for explaining the unusual behavior of many materials. These materials are interesting both from a fundamental view point and for application to future technologies. One of the simplest many-body phenomena is the interaction of a local "impurity" spin with a sea of electrons, the so-called "Kondo Impurity Problem," discovered about half a century ago. In the last two decades there has been a huge revival in the study of "Kondo" type phenomena. Experiments on two types of quantum materials have been responsible for this revival. On the one hand, fabrication of nano-meter scale electronic devices that act as "Kondo" impurities have provided flexible and tunable realizations of quantum impurities. On the other hand, the discovery of "Kondo" lattice materials (or "Heavy-Fermion" metals) have provided a window onto the physics of metals with a dense concentration of "Kondo" impurities. This thesis is concerned with physical problems relevant to both these types of materials. Part I of this thesis is concerned with manifestations of the interplay of quantum coherence and the Kondo effect in nano-structures. The effect of this interesting competition can be observed in a variety of nano-devices. In some set-ups the Kondo temperature itself becomes a mesoscopic quantity (Chapter 3), exhibiting huge sample to sample fluctuations, while in other set-ups the definition of the Kondo temperature itself becomes the question of interest (Chapter 4). We have also developed a new method to simulate general quantum impurity models using quantum Monte-Carlo methods (Chapter 5) and applied it to study the universal Kondo physics that takes place when the screening bath is placed in a finite-size box. Finally, we have proposed a new experimental set-up in which the finite-size spectrum of many interesting quantum impurity problems

  19. Kondo force in shuttling devices: dynamical probe for a Kondo cloud.

    PubMed

    Kiselev, M N; Kikoin, K A; Gorelik, L Y; Shekhter, R I

    2013-02-08

    We consider the electromechanical properties of a single-electronic device consisting of a movable quantum dot attached to a vibrating cantilever, forming a tunnel contact with a nonmovable source electrode. We show that the resonance Kondo tunneling of electrons amplifies exponentially the strength of nanoelectromechanical (NEM) coupling in such a device and make the latter insensitive to mesoscopic fluctuations of electronic levels in a nanodot. It is also shown that the study of a Kondo-NEM phenomenon provides additional (as compared with standard conductance measurements in a nonmechanical device) information on retardation effects in the formation of a many-particle cloud accompanying the Kondo tunneling. A possibility for superhigh tunability of mechanical dissipation as well as supersensitive detection of mechanical displacement is demonstrated.

  20. Competing Kondo Effects in Non-Kramers Doublet Systems

    NASA Astrophysics Data System (ADS)

    Kusunose, Hiroaki

    2016-06-01

    In non-Kramers Kondo systems with quadrupolar degrees of freedom, an ordinary magnetic Kondo effect can compete with the quadrupolar Kondo effect. We discuss such competition keeping PrT2Zn20 (T = Ir, Rh) and PrT2Al20 (T = V, Ti) in mind, where the Γ3 non-Kramers crystalline-electric-field (CEF) doublet ground state is realized in a Pr3+ ion with a (4f)2 configuration under cubic symmetry. The quadrupolar Kondo effect can be described by the two-channel Kondo model, which leads to the local non-Fermi-liquid (NFL) ground state, while the magnetic Kondo effect favors the ordinary local Fermi-liquid (FL) ground state. On the basis of the minimal extended two-channel Kondo model including the magnetic Kondo coupling as well, we investigate the competition and resulting thermodynamics, and orbital/magnetic and single-particle excitation spectra by Wilson's numerical renormalization group (NRG) method. There is a first-order transition between the NFL and FL ground states. In addition to these two states, the alternative FL state accompanied by a free magnetic spin appears in the intermediate temperature range, which eventually reaches the true NFL ground state, as a consequence of the stronger competition between the magnetic and quadrupolar Kondo effects. In this peculiar state, the magnetic susceptibility shows a Curie-like behavior, while the orbital fluctuation exhibits the FL behavior. Moreover, the single-particle spectra yield a more singular behavior. Implications to the Pr 1-2-20 systems are briefly discussed.

  1. Evidence of Kondo effect in organic radical nanoassemblies

    NASA Astrophysics Data System (ADS)

    Rashidi, Mohammad; Mullegger, Stefan; Fattinger, Michael; Koch, Reinhold

    2012-02-01

    The outstanding spatial resolution of low temperature (LT) scanning tunneling microscopy (STM) and spectroscopy (STS) enables to probe the frontier orbital electronic structure of single magnetic molecules and clusters adsorbed on substrates. Here, we study self-aligned nanostructures of (spin-1/2) hydrocarbon radicals on a metal surface by means of LT-STM and STS. Pronounced involvement of surface state electrons is observed in the frontier molecular orbital (MO) resonances. An empty hybrid state closely above the substrate Fermi level exhibits the characteristic properties of surface Kondo effect reported for similar systems in the literature. By identifying three electronic states as hybrids of molecular orbitals and surface state electrons (two of them directly related to the Kondo effect), we are able to present a modified picture of the surface Kondo effect. It is based on a valence-bond model, where the bonding state represents Kondo's virtual bound state and the antibonding state is the so called 'Kondo resonance' reported in STM studies of the surface Kondo effect. Furthermore, double occupation of the originally singly unoccupied MO by tunneling electrons leads to the third state well above the Fermi level due to Coulomb repulsion as described by the Anderson model.

  2. Entanglement entropy near Kondo-destruction quantum critical points

    NASA Astrophysics Data System (ADS)

    Chowdhury, Tathagata; Wagner, Christopher; Ingersent, Kevin; Pixley, Jedediah

    Entanglement entropy is a measure of quantum-mechanical entanglement across the boundary created by partitioning a system into two subsystems. We study this quantity in Kondo impurity models that feature Kondo-destruction quantum critical points (QCPs). Recent work has shown that the entanglement entropy between a Kondo impurity of spin Simp and its environment is pinned at its maximum possible value Se = ln (2Simp + 1) throughout the Kondo phase. In the Kondo-destroyed phase, where the impurity spin acquires a nonzero expectation value Mloc, Se = ln (2Simp + 1) - a (Simp) Mloc2 irrespective of the properties of the host. Here, we report numerical renormalization-group results for Kondo models with a pseudogapped density of states under a different partition that separates the impurity and on-site conduction electrons from the rest of the system. Now, the entanglement entropy is affected by the nature of the environment beyond the information contained in Mloc, but Se still contains a critical part that exhibits power-law behavior in the vicinity of the Kondo-destruction QCP

  3. Periodically driven Kondo impurity in nonequilibrium steady states

    NASA Astrophysics Data System (ADS)

    Iwahori, Koudai; Kawakami, Norio

    2016-12-01

    We study the nonequilibrium dynamics of a periodically driven anisotropic Kondo impurity model. The periodic time dependence is introduced for a local magnetic field which couples to the impurity spin and also for an in-plane exchange interaction. We obtain the exact results on the time evolution for arbitrary periodic time dependence at the special point in the parameter space known as the Toulouse limit. We first consider a specific case where the local magnetic field is periodically switched on and off. When the driving period is much shorter than the inverse of the Kondo temperature, an intriguing oscillating behavior (resonance phenomenon) emerges in the time average of the impurity spin polarization with increasing the local magnetic field intensity. By taking the high-frequency limit of the external driving, we elucidate that the system recovers the translational invariance in time and can be described by a mixture of the zero-temperature and infinite-temperature properties. In certain cases, the system is governed by either zero-temperature or infinite-temperature properties and, therefore, can be properly described by the corresponding equilibrium state.

  4. Kondo lattice and antiferromagnetic behavior in quaternary CeTAl4Si2 (T = Rh, Ir) single crystals

    SciTech Connect

    Maurya, Arvind; Kulkarni, Ruta; Thamizhavel, Arumugam; Paudyal, Durga; Dhar, Sudesh Kumar

    2016-02-26

    Here, we have explored in detail the anisotropic magnetic properties of CeRhAl4Si2 and CeIrAl4Si2, which undergo two antiferromagnetic transitions, at TN1 = 12.6 and 15.5 K, followed by a second transition at TN2 = 9.4 and 13.8 K, respectively, with the [001]-axis as the relatively easy axis of magnetization. The electrical resistivity at ambient and applied pressure provides evidence of Kondo interaction in both compounds, further supported by a reduced value of the entropy associated with the magnetic ordering. The Sommerfeld coefficient γ is inferred to be 195.6 and 49.4 mJ/(mol K2) for CeRhAl4Si2 and CeIrAl4Si2, respectively, classifying these materials as moderate heavy-fermion compounds. The crystal electric field energy levels are derived from the peak seen in the Schottky heat capacity. Furthermore, we have also performed electronic structure calculations by using the local spin density approximation + U [LSDA+U] approach, which provide physical insights on the observed magnetic behavior of these two compounds.

  5. Competition between Kondo Screening and Quantum Hall Edge Reconstruction

    NASA Astrophysics Data System (ADS)

    Heine, A. W.; Tutuc, D.; Zwicknagl, G.; Haug, R. J.

    2016-03-01

    We report on a Kondo correlated quantum dot connected to two-dimensional leads where we demonstrate the renormalization of the g factor in the pure Zeeman case. i.e., for magnetic fields parallel to the plane of the quantum dot. For the same system, we study the influence of orbital effects by investigating the quantum Hall regime; i.e., a perpendicular magnetic field is applied. In this case an unusual behavior of the suppression of the Kondo effect and of the split zero-bias anomaly is observed. The splitting decreases with magnetic field and shows discontinuous changes that are attributed to the intricate interplay between Kondo screening and the quantum Hall edge structure originating from electrostatic screening. This edge structure, made up of compressible and incompressible stripes, strongly affects the Kondo temperature of the quantum dot and thereby influences the renormalized g factor.

  6. Fano–Andreev effect in a T-shape double quantum dot in the Kondo regime

    NASA Astrophysics Data System (ADS)

    Calle, A. M.; Pacheco, M.; Martins, G. B.; Apel, V. M.; Lara, G. A.; Orellana, P. A.

    2017-04-01

    In the present work, we investigate the electronic transport through a T-shape double quantum dot system coupled to two normal leads and to one superconducting lead. We explore the interplay between Kondo and Andreev states due to proximity effects. We find that Kondo resonance is modified by the Andreev bound states, which manifest through Fano antiresonances in the local density of states of the embedded quantum dot and normal transmission. This means that there is a correlation between Andreev bound states and Fano resonances that is robust under the influence of high electronic correlation. We have also found that the dominant couplings at the quantum dots are characterized by a crossover region that defines the range where the Fano–Kondo and the Andreev–Kondo effect prevail in each quantum dot. Likewise, we find that the interaction between Kondo and Andreev bound states has a notable influence on the Andreev transport.

  7. Two-point functions in a holographic Kondo model

    NASA Astrophysics Data System (ADS)

    Erdmenger, Johanna; Hoyos, Carlos; O'Bannon, Andy; Papadimitriou, Ioannis; Probst, Jonas; Wu, Jackson M. S.

    2017-03-01

    We develop the formalism of holographic renormalization to compute two-point functions in a holographic Kondo model. The model describes a (0 + 1)-dimensional impurity spin of a gauged SU( N ) interacting with a (1 + 1)-dimensional, large- N , strongly-coupled Conformal Field Theory (CFT). We describe the impurity using Abrikosov pseudo-fermions, and define an SU( N )-invariant scalar operator O built from a pseudo-fermion and a CFT fermion. At large N the Kondo interaction is of the form O^{\\dagger}O, which is marginally relevant, and generates a Renormalization Group (RG) flow at the impurity. A second-order mean-field phase transition occurs in which O condenses below a critical temperature, leading to the Kondo effect, including screening of the impurity. Via holography, the phase transition is dual to holographic superconductivity in (1 + 1)-dimensional Anti-de Sitter space. At all temperatures, spectral functions of O exhibit a Fano resonance, characteristic of a continuum of states interacting with an isolated resonance. In contrast to Fano resonances observed for example in quantum dots, our continuum and resonance arise from a (0 + 1)-dimensional UV fixed point and RG flow, respectively. In the low-temperature phase, the resonance comes from a pole in the Green's function of the form - i< O >2, which is characteristic of a Kondo resonance.

  8. Kondo screening of the spin and orbital magnetic moments of Fe impurities in Cu

    NASA Astrophysics Data System (ADS)

    Joly, L.; Kappler, J.-P.; Ohresser, P.; Sainctavit, Ph.; Henry, Y.; Gautier, F.; Schmerber, G.; Kim, D. J.; Goyhenex, C.; Bulou, H.; Bengone, O.; Kavich, J.; Gambardella, P.; Scheurer, F.

    2017-01-01

    We use x-ray magnetic circular dichroism to evidence the effect of correlations on the local impurity magnetic moment in an archetypal Kondo system, namely, a dilute Cu:Fe alloy. Applying the sum rules on the Fe L2 ,3 absorption edges, the evolution of the spin and orbital moments across the Kondo temperature are determined separately. The spin moment presents a crossover from a nearly temperature-independent regime below the Kondo temperature to a paramagneticlike regime above. Conversely, the weak orbital moment shows a temperature-independent behavior in the whole temperature range, suggesting different Kondo screening temperature scales for the spin and orbital moments.

  9. Mid-gap states and Kondo effect in disordered graphene

    NASA Astrophysics Data System (ADS)

    Lewenkopf, Caio; Miranda, Vladimir; Dias da Silva, Luis

    2012-02-01

    Recent experiments on graphene flakes with short range scattering defects have stengthen the interest on Kondo physics in graphene systems. The experimental data show a temperature dependence of the resistivity consistent with the low-temperature Kondo screening of local magnetic moments. While the linear dispersion in the density of states in graphene justify a pseudogap Kondo model showing a rich variety of quantum critical behavior as a function of the gate-controlled chemical potential, the presence of disorder can alter this effect in favor of the ``standard'' Kondo model, with a Fermi-liquid ground state. We study these effects with different numerical methods. Tight-binding calculations for diluted scattering defects show the appearance of quasi-localized midgap states in the local density of states at the vicinity of the charge neutrality point. This leads to the formulation a Anderson-like model of localized states within the graphene matrix, which may lead to a Kondo screening consistent with the experiments. To verify this hypothesis, we perform numerical renormalization group (NRG) calculations to study the gate-dependence of the Kondo temperature and the transport properties of this model.

  10. Panel resonant behavior of wind turbine blades.

    SciTech Connect

    Paquette, Joshua A.; Griffith, Daniel Todd

    2010-03-01

    The principal design drivers in the certification of wind turbine blades are ultimate strength, fatigue resistance, adequate tip-tower clearance, and buckling resistance. Buckling resistance is typically strongly correlated to both ultimate strength and fatigue resistance. A composite shell with spar caps forms the airfoil shape of a blade and reinforcing shear webs are placed inside the blade to stiffen the blade in the flap-wise direction. The spar caps are dimensioned and the shear webs are placed so as to add stiffness to unsupported panel regions and reduce their length. The panels are not the major flap-wise load carrying element of a blade; however, they must be designed carefully to avoid buckling while minimizing blade weight. Typically, buckling resistance is evaluated by consideration of the load-deflection behavior of a blade using finite element analysis (FEA) or full-scale static testing of blades under a simulated extreme loading condition. The focus of this paper is on the use of experimental modal analysis to measure localized resonances of the blade panels. It can be shown that the resonant behavior of these panels can also provide a means to evaluate buckling resistance by means of analytical or experimental modal analysis. Further, panel resonances have use in structural health monitoring by observing changes in modal parameters associated with panel resonances, and use in improving panel laminate model parameters by correlation with test data. In recent modal testing of wind turbine blades, a set of panel modes were measured. This paper will report on the findings of these tests and accompanying numerical and analytical modeling efforts aimed at investigating the potential uses of panel resonances for blade evaluation, health monitoring, and design.

  11. Spin polarization of the split Kondo state.

    PubMed

    von Bergmann, Kirsten; Ternes, Markus; Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

    2015-02-20

    Spin-resolved scanning tunneling microscopy is employed to quantitatively determine the spin polarization of the magnetic field-split Kondo state. Tunneling conductance spectra of a Kondo-screened magnetic atom are evaluated within a simple model taking into account inelastic tunneling due to spin excitations and two Kondo peaks positioned symmetrically around the Fermi energy. We fit the spin state of the Kondo-screened atom with a spin Hamiltonian independent of the Kondo effect and account for Zeeman splitting of the Kondo peak in the magnetic field. We find that the width and the height of the Kondo peaks scales with the Zeeman energy. Our observations are consistent with full spin polarization of the Kondo peaks, i.e., a majority spin peak below the Fermi energy and a minority spin peak above.

  12. Analysis of the antiferromagnetic phase transitions of the 2D Kondo lattice

    NASA Astrophysics Data System (ADS)

    Jones, Barbara

    2010-03-01

    The Kondo lattice continues to present an interesting and relevant challenge, with its interactions between Kondo, RKKY, and coherent order. We present our study[1] of the antiferromagnetic quantum phase transitions of a 2D Kondo-Heisenberg square lattice. Starting from the nonlinear sigma model as a model of antiferromagnetism, we carry out a renormalization group analysis of the competing Kondo-RKKY interaction to one-loop order in an ɛ-expansion. We find a new quantum critical point (QCP) strongly affected by Kondo fluctuations. Near this QCP, there is a breakdown of hydrodynamic behavior, and the spin waves are logarithmically frozen out. The renormalization group results allow us to propose a new phase diagram near the antiferromagnetic fixed point of this 2D Kondo lattice model. The T=0 phase diagram contains four phases separated by a tetracritical point, the new QCP. For small spin fluctuations, we find a stable local magnetic moment antiferromagnet. For stronger coupling, region II is a metallic quantum disordered paramagnet. We find in region III a paramagnetic phase driven by Kondo interactions, with possible ground states of a heavy fermion liquid or a Kondo driven spin-liquid. The fourth phase is a spiral phase, or a large-Fermi-surface antiferromagnetic phase. We will describe these phases in more detail, including possible experimental confirmation of the spiral phase. The existence of the tetracritical point found here would be expected to affect the phase diagram at finite temperatures as well. In addition, It is hoped that these results, and particularly the Kondo interaction paramagnetic phase, will serve to bridge to solutions starting from the opposite limit, of a Kondo effect leading to a heavy fermion ground state. Work in collaboration with T. Tzen Ong. [4pt] [1] T. Ong and B. A. Jones, Phys. Rev. Lett. 103, 066405 (2009).

  13. A maximally supersymmetric Kondo model

    NASA Astrophysics Data System (ADS)

    Harrison, Sarah; Kachru, Shamit; Torroba, Gonzalo

    2012-10-01

    We study the maximally supersymmetric Kondo model obtained by adding a fermionic impurity to N=4 supersymmetric Yang-Mills theory. While the original Kondo problem describes a defect interacting with a free Fermi liquid of itinerant electrons, here the ambient theory is an interacting CFT, and this introduces qualitatively new features into the system. The model arises in string theory by considering the intersection of a stack of M D5-branes with a stack of N D3-branes, at a point in the D3 worldvolume. We analyze the theory holographically, and propose a dictionary between the Kondo problem and antisymmetric Wilson loops in N=4 SYM. We perform an explicit calculation of the D5 fluctuations in the D3 geometry and determine the spectrum of defect operators. This establishes the stability of the Kondo fixed point together with its basic thermodynamic properties. Known supergravity solutions for Wilson loops allow us to go beyond the probe approximation: the D5s disappear and are replaced by three-form flux piercing a new topologically non-trivial S3 in the corrected geometry. This describes the Kondo model in terms of a geometric transition. A dual matrix model reflects the basic properties of the corrected gravity solution in its eigenvalue distribution.

  14. A Maximally Supersymmetric Kondo Model

    SciTech Connect

    Harrison, Sarah; Kachru, Shamit; Torroba, Gonzalo; /Stanford U., Phys. Dept. /SLAC

    2012-02-17

    We study the maximally supersymmetric Kondo model obtained by adding a fermionic impurity to N = 4 supersymmetric Yang-Mills theory. While the original Kondo problem describes a defect interacting with a free Fermi liquid of itinerant electrons, here the ambient theory is an interacting CFT, and this introduces qualitatively new features into the system. The model arises in string theory by considering the intersection of a stack of M D5-branes with a stack of N D3-branes, at a point in the D3 worldvolume. We analyze the theory holographically, and propose a dictionary between the Kondo problem and antisymmetric Wilson loops in N = 4 SYM. We perform an explicit calculation of the D5 fluctuations in the D3 geometry and determine the spectrum of defect operators. This establishes the stability of the Kondo fixed point together with its basic thermodynamic properties. Known supergravity solutions for Wilson loops allow us to go beyond the probe approximation: the D5s disappear and are replaced by three-form flux piercing a new topologically non-trivial S3 in the corrected geometry. This describes the Kondo model in terms of a geometric transition. A dual matrix model reflects the basic properties of the corrected gravity solution in its eigenvalue distribution.

  15. Emergence of a Kondo singlet state with Kondo temperature well beyond 1000 K in a proton-embedded electron gas

    NASA Astrophysics Data System (ADS)

    Takada, Yasutami; Maezono, Ryo; Yoshizawa, Kanako

    2015-10-01

    Hydrogen in metals has attracted much attention for a long time from both basic scientific and technological points of view. Its electronic state has been investigated in terms of a proton embedded in the electron gas mostly by the local density approximation (LDA) to the density functional theory. At high electronic densities, it is well described by a bare proton H+ screened by metallic electrons (charge resonance), while at low densities two electrons are localized at the proton site to form a closed-shell negative ion H- protected from surrounding metallic electrons by the Pauli exclusion principle. However, no details are known about the transition from H+ to H- in the intermediate-density region. Here, by accurately determining the ground-state electron distribution n (r ) by the use of LDA and diffusion Monte Carlo simulations with the total electron number up to 170, we obtain a complete picture of the transition, in particular, a sharp transition from short-range H+ screening charge resonance to long-range Kondo-type spin-singlet resonance, the emergence of which is confirmed by the presence of an anomalous Friedel oscillation characteristic to the Kondo singlet state with the Kondo temperature TK well beyond 1000 K. This study not only reveals interesting competition between charge and spin resonances, enriching the century-old paradigm of metallic screening to a point charge, but also discovers a high-TK system long sought in relation to the development of exotic superconductivity in the quantum critical regime.

  16. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: Kondo effect in a deformed molecule coupled asymmetrically to ferromagnetic electrodes

    NASA Astrophysics Data System (ADS)

    Wang, Rui-Qiang; Jiang, Kai-Ming

    2009-12-01

    The nonequilibrium Kondo effect is studied in a molecule quantum dot coupled asymmetrically to two ferromagnetic electrodes by employing the nonequilibrium Green function technique. The current-induced deformation of the molecule is taken into account, modeled as interactions with a phonon system, and phonon-assisted Kondo satellites arise on both sides of the usual main Kondo peak. In the antiparallel electrode configuration, the Kondo satellites can be split only for the asymmetric dot-lead couplings, distinguished from the parallel configuration where splitting also exists, even though it is for symmetric case. We also analyze how to compensate the splitting and restore the suppressed zero-bias Kondo resonance. It is shown that one can change the TMR ratio significantly from a negative dip to a positive peak only by slightly modulating a local external magnetic field, whose value is greatly dependent on the electron-phonon coupling strength.

  17. Kondo effect in a quantum dot side-coupled to a topological superconductor

    NASA Astrophysics Data System (ADS)

    Lee, Minchul; Lim, Jong Soo; López, Rosa

    2013-06-01

    We investigate the dynamical and transport features of a Kondo dot side coupled to a topological superconductor (TS). The Majorana fermion states (MFSs) formed at the ends of the TS are found to be able to alter the Kondo physics profoundly: For an infinitely long wire where the MFSs do not overlap (ɛm=0) a finite dot-MFS coupling (Γm) reduces the unitary-limit value of the linear conductance by exactly a factor 3/4 in the weak-coupling regime (ΓmKondo temperature. In the strong-coupling regime (Γm>TK), on the other hand, the spin-split Kondo resonance takes place due to the MFS-induced Zeeman splitting, which is a genuine many-body effect of the strong Coulomb interaction and the topological superconductivity. We find that the original Kondo resonance is fully restored once the MFSs are strongly hybridized (ɛm>Γm). This unusual interaction between the Kondo effect and the MFS can thus serve to detect the Majorana fermions unambiguously and quantify the degree of overlap between the MFSs in the TS.

  18. Magnetic excitations in the kondo liquid: superconductivity and hidden magnetic quantum critical fluctuations.

    PubMed

    Yang, Yi-Feng; Urbano, Ricardo; Curro, Nicholas J; Pines, David; Bauer, E D

    2009-11-06

    We report Knight-shift experiments on the superconducting heavy-electron material CeCoIn5 that allow one to track with some precision the behavior of the heavy-electron Kondo liquid in the superconducting state with results in agreement with BCS theory. An analysis of the 115In nuclear quadrupole resonance spin-lattice relaxation rate T1(-1) measurements under pressure reveals the presence of 2d magnetic quantum critical fluctuations in the heavy-electron component that are a promising candidate for the pairing mechanism in this material. Our results are consistent with an antiferromagnetic quantum critical point located at slightly negative pressure in CeCoIn5 and provide additional evidence for significant similarities between the heavy-electron materials and the high-T(c) cuprates.

  19. Emergence of a Fermionic Finite-Temperature Critical Point in a Kondo Lattice.

    PubMed

    Chou, Po-Hao; Zhai, Liang-Jun; Chung, Chung-Hou; Mou, Chung-Yu; Lee, Ting-Kuo

    2016-04-29

    The underlying Dirac point is central to the profound physics manifested in a wide class of materials. However, it is often difficult to drive a system with Dirac points across the massless fermionic critical point. Here by exploiting screening of local moments under spin-orbit interactions in a Kondo lattice, we show that below the Kondo temperature, the Kondo lattice undergoes a topological transition from a strong topological insulator to a weak topological insulator at a finite temperature T_{D}. At T_{D}, massless Dirac points emerge and the Kondo lattice becomes a Dirac semimetal. Our analysis indicates that the emergent relativistic symmetry dictates nontrivial thermal responses over large parameter and temperature regimes. In particular, it yields critical scaling behaviors both in magnetic and transport responses near T_{D}.

  20. Coupled Quantum Dots in the Kondo regime: interference and filtering effects.

    NASA Astrophysics Data System (ADS)

    Dias da Silva, Luis; Sandler, Nancy; Ingersent, Kevin; Ulloa, Sergio

    2006-03-01

    Double quantum-dot systems (DQDs) provide a vast array of possibilities for both theoretical and experimental investigations of the Kondo regime. In this work, we propose DQDs as a possible experimental realization of a Kondo impurity coupled to an effective structured (non-constant) density of states (DoS). We consider a DQD in parallel configuration coupled to metallic leads. By changing the lead-dot and dot-dot couplings, the effective hybridization function for an individual dot displays sharp resonances and/or pseudogaps, allowing for an experimental probe into the transition between both regimes. Using numerical renormalization group methods, we calculate the dot's spectral function in different regimes. For a dot weakly coupled to the leads and strongly coupled to the second dot, the effective DoS has a sharp resonance with width δ and the spectral density shows a splitting in the Kondo resonance for TK>δ, although the Kondo singlet is preserved. Furthermore, for small inter-dot coupling, second order dot-dot interactions through the conduction electrons lead to the formation of a pseudo-gap. The spectral density goes to zero as a power-law |ɛ-ɛF|^2 and the Kondo screening is suppressed. Supported by NFS-NIRT.

  1. Kondo effect in bosonic spin liquids.

    PubMed

    Florens, Serge; Fritz, Lars; Vojta, Matthias

    2006-01-27

    In a metal, a magnetic impurity is fully screened by the conduction electrons at low temperature. In contrast, impurity moments coupled to spin-1 bulk bosons, such as triplet excitations in paramagnets, are only partially screened, even at the bulk quantum critical point. We argue that this difference is not due to the quantum statistics of the host particles but instead related to the structure of the impurity-host coupling, by demonstrating that frustrated magnets with bosonic spinon excitations can display a bosonic version of the Kondo effect. However, the Bose statistics of the bulk implies distinct behavior, such as a weak-coupling impurity quantum phase transition, and perfect screening for a range of impurity spin values. We discuss implications of our results for the compound Cs2CuCl4, as well as possible extensions to multicomponent bosonic gases.

  2. Toward a new microscopic framework for Kondo lattice materials

    NASA Astrophysics Data System (ADS)

    Lonzarich, Gilbert; Pines, David; Yang, Yi-feng

    2017-02-01

    Understanding the emergence and subsequent behavior of heavy electrons in Kondo lattice materials is one of the grand challenges in condensed matter physics. From this perspective we review the progress that has been made during the past decade and suggest some directions for future research. Our focus will be on developing a new microscopic framework that incorporates the basic concepts that emerge from a phenomenological description of the key experimental findings.

  3. Preserved Kondo effect of small cobalt atomic chains on Ru(0001) surface

    NASA Astrophysics Data System (ADS)

    Feng, Wei; Liu, Qin; Zhou, Chunsheng; Lai, Xinchun; Li, Bin; Zhao, Aidi

    2016-12-01

    The evolution of the Kondo effect from a cobalt monomer to a compact dimer, a linear trimer and then a triangular trimer on Ru(0001) surface was studied by atomic manipulation and scanning tunneling spectroscopy (STS). It is found that the Kondo resonances of a compact Co dimer and linear trimer still can be detected in their STS because of the weak ferromagnetic exchange interaction between the Co atoms. However, when the number of the nearest-neighbors for every Co atom in the compact Co clusters is larger than one, for the interaction between Co atoms enter into the regime of the strong ferromagnetic exchange interaction, the Kondo resonance disappear and a new state forms.

  4. Macroscopic quantum entanglement of a Kondo cloud at finite temperature.

    PubMed

    Lee, S-S B; Park, Jinhong; Sim, H-S

    2015-02-06

    We propose a variational approach for computing the macroscopic entanglement in a many-body mixed state, based on entanglement witness operators, and compute the entanglement of formation (EoF), a mixed-state generalization of the entanglement entropy, in single- and two-channel Kondo systems at finite temperature. The thermal suppression of the EoF obeys power-law scaling at low temperature. The scaling exponent is halved from the single- to the two-channel system, which is attributed, using a bosonization method, to the non-Fermi liquid behavior of a Majorana fermion, a "half" of a complex fermion, emerging in the two-channel system. Moreover, the EoF characterizes the size and power-law tail of the Kondo screening cloud of the single-channel system.

  5. Conductance fingerprint of Majorana fermions in the topological Kondo effect

    NASA Astrophysics Data System (ADS)

    Galpin, Martin R.; Mitchell, Andrew K.; Temaismithi, Jesada; Logan, David E.; Béri, Benjamin; Cooper, Nigel R.

    2014-01-01

    We consider an interacting nanowire/superconductor heterostructure attached to metallic leads. The device is described by an unusual low-energy model involving spin-1 conduction electrons coupled to a nonlocal spin-1/2 Kondo impurity built from Majorana fermions. The topological origin of the resulting Kondo effect is manifest in distinctive non-Fermi-liquid (NFL) behavior, and the existence of Majorana fermions in the device is demonstrated unambiguously by distinctive conductance line shapes. We study the physics of the model in detail, using the numerical renormalization group, perturbative scaling, and Abelian bosonization. In particular, we calculate the full scaling curves for the differential conductance in ac and dc fields, onto which experimental data should collapse. Scattering t matrices and thermodynamic quantities are also calculated, recovering asymptotes from conformal field theory. We show that the NFL physics is robust to asymmetric Majorana-lead couplings, and here we uncover a duality between strong and weak coupling. The NFL behavior is understood physically in terms of competing Kondo effects. The resulting frustration is relieved by inter-Majorana coupling which generates a second crossover to a regular Fermi liquid.

  6. Two-channel Kondo physics in a Majorana island coupled to a Josephson junction

    NASA Astrophysics Data System (ADS)

    Landau, L. A.; Sela, E.

    2017-01-01

    We study a Majorana island coupled to a bulk superconductor via a Josephson junction and to multiple external normal leads. In the absence of the Josephson coupling, the system displays a topological Kondo state, which had been largely studied recently. However, we find that this state is unstable even to small Josephson coupling, which instead leads at low temperature T to a new fixed point. Most interesting is the case of three external leads, forming a minimal electronic realization of the long sought two-channel Kondo effect. While the T =0 conductance corresponds to simple resonant Andreev reflection, the leading T dependence forms an experimental fingerprint for non-Fermi-liquid properties.

  7. Magnetic field induced mixed level Kondo effect in two-level quantum dots

    NASA Astrophysics Data System (ADS)

    Wong, Arturo; Ngo, Anh; Ulloa, Sergio

    2012-02-01

    Semiconductor quantum dots provide an easily tunable environment in which to investigate the Kondo effect. As it is known, Kondo correlations are suppressed by magnetic fields, showing e.g. a drop in the conductance of a quantum dot device. However, certain systems may exhibit an increasing conductance as a function of an applied magnetic field [1]. In this work we use the numerical renormalization group method to study a two-level quantum dot system with on-level and interlevel Coulomb repulsion, coupled to a single channel. When there is a finite detuning between levels, and a local singlet develops in one of them, the linear conductance of the device shows a maximum structure as a function of an in-plane magnetic field, which depends on the temperature of the system. This maximum occurs at a magnetic field strength such that the spin up state of one of the levels and spin down of the other are degenerate, allowing a ``mixed level'' Kondo effect. The respective spectral functions feature a resonance at the Fermi energy, commensurate with the Kondo physics. We discuss the properties of this mixed level Kondo state in terms of the detuning and the other parameters of the system. [4pt] [1] R. Sakano and N. Kawakami, PRB 73, 155332 (2006)

  8. Quantum dots with even number of electrons: kondo effect in a finite magnetic field

    PubMed

    Pustilnik; Avishai; Kikoin

    2000-02-21

    We show that the Kondo effect can be induced by an external magnetic field in quantum dots with an even number of electrons. If the Zeeman energy B is close to the single-particle level spacing Delta in the dot, the scattering of the conduction electrons from the dot is dominated by an anisotropic exchange interaction. A Kondo resonance then occurs despite the fact that B exceeds by far the Kondo temperature T(K). As a result, at low temperatures T

  9. Kondo interactions from band reconstruction in YbInCu4

    DOE PAGES

    Jarrige, I.; Kotani, A.; Yamaoka, H.; ...

    2015-03-27

    We combine resonant inelastic X-ray scattering (RIXS) and model calculations in the Kondo lattice compound YbInCu₄, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T≃42 K. In this study, the bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasi-gap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system.

  10. Low temperature properties of the Kondo insulator FeSi

    NASA Astrophysics Data System (ADS)

    Figueira, M. S.; Franco, R.

    2007-07-01

    In this paper we study the low temperature (T) properties of the Kondo insulator FeSi within the X-boson approach. We show that the ground state of the FeSi is metallic and highly correlated with a large effective mass; the low temperature contributions to the specific heat and the resistivity are of the Fermi-liquid type. The low temperature properties are governed by a reentrant transition into a metallic state, that occurs when the chemical potential crosses the gap and enters the conduction band, generating a metallic ground state. The movement of the chemical potential is due to the strong correlations present in the system. We consider the low temperature regime of the Kondo insulator FeSi, where the hybridization gap is completely open. In this situation we identify the two characteristic temperatures: the coherence temperature T0 and the Kondo temperature TKL. In the range T < T0, we identify a regime characterized by the formation of coherent states and Fermi-liquid behavior of the low temperature properties; in the range TKL > T > T0, we identify a regime characterized by an activation energy. Within the X-boson approach we study those low temperature regimes although we do not try to adjust parameters to recover the experimental energy scales.

  11. The low temperature spectral weight transfer problem in Kondo insulators

    NASA Astrophysics Data System (ADS)

    Franco, R.; Silva-Valencia, J.; Figueira, M. S.

    2009-01-01

    In this paper we address the problem of the spectral weight transfer in Kondo insulators (KI). We employ the X-boson approach for the periodic Anderson model, in the U →∞ limit. We calculate the two energy gaps of the system analytically: the indirect gap, Δind = Eg ≃ Emir, present in the density of states, and the direct one Δdir, associated with the minimum energy necessary to produce inter-band transitions. We find that the optical behavior of the system is governed by two energy scales: one of low frequency, characterized by Eg ≃ Emir, in the mid-infrared region (MIR), which is a reminiscent of the heavy fermion Emir peak, that appears in Kondo insulators as a broad maximum in the MIR region and that controls the low temperature transport properties, the gap opening in optical conductivity and the formation of the Drude peak, at ω = 0, in the intermediate temperature range. The other energy scale appears at high frequencies, and is characterized by the direct gap Δdir. According to our results, this peak controls the anomalous redistribution of spectral weight in the optical conductivity. We apply the theory in order to study the Kondo insulator FeSi, and we calculate the optical conductivity of the system and the spectral weight transfer in the optical conductivity.

  12. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: Splitting and Restoration of Kondo Peak in a Deformed Molecule Quantum Dot Coupled to Ferromagnetic Electrodes

    NASA Astrophysics Data System (ADS)

    Wang, Rui-Qiang; Jiang, Kai-Ming

    2010-02-01

    We adopt the nonequilibrium Green's function method to theoretically study the Kondo effect in a deformed molecule, which is treated as an electron-phonon interaction (EPI) system. The self-energy for phonon part is calculated in the standard many-body diagrammatic expansion up to the second order in EPI strength. We find that the multiple phonon-assisted Kondo satellites arise besides the usual Kondo resonance. In the antiparallel magnetic configuration the splitting of main Kondo peak and phonon-assisted satellites only happen for asymmetrical dot-lead couplings, but it is free from the symmetry for the parallel magnetic configuration. The EPI strength and vibrational frequency can enhance the spin splitting of both main Kondo and satellites. It is shown that the suppressed zero-bias Kondo resonance can be restored by applying an external magnetic field, whose magnitude is dependent on the phononic effect remarkably. Although the asymmetry in tunnel coupling has no contribution to the restoration of spin splitting of Kondo peak, it can shrink the external field needed to switch tunneling magnetoresistance ratio between large negative dip and large positive peak.

  13. The Kondo necklace model with planar anisotropy

    NASA Astrophysics Data System (ADS)

    Mendoza-Arenas, J. J.; Franco, R.; Silva-Valencia, J.

    2009-10-01

    We study the one-dimensional anisotropic Kondo necklace model at zero temperature through White's density matrix renormalization group technique. The ground state energy and the spin gap were calculated as a function of the exchange parameter for two anisotropy values. We found a finite critical point separating a Kondo singlet from an antiferromagnetic phase. The transition is highly congruent with a Kosterlitz-Thouless form. We observed that the critical point increases with the anisotropy.

  14. Collapse of the G d3 + ESR fine structure throughout the coherent temperature of the Gd-doped Kondo Semiconductor CeF e4P12

    NASA Astrophysics Data System (ADS)

    Venegas, P. A.; Garcia, F. A.; Garcia, D. J.; Cabrera, G. G.; Avila, M. A.; Rettori, C.

    2016-12-01

    Recent experiments on G d3 + electron-spin resonance (ESR) in the filled skutterudite C e1 -xG dxF e4P12(x ≈0.001 ) , at temperatures where the host resistivity manifests a smooth insulator-metal crossover, provide evidence of the underlying Kondo physics associated with this system. At low temperatures (below T ≈160 K), C e1 -xG dxF e4P12 behaves as a Kondo insulator with a relatively large hybridization gap, and the G d3 + ESR spectra display a fine structure with Lorentzian line shape, typical of insulating media. In this work, based on previous experiments performed by the same group, we argue that the electronic gap may be attributed to the large hybridization present in the coherent regime of a Kondo lattice. Moreover, mean-field calculations suggest that the electron-phonon interaction is fundamental at explaining such hybridization. The resulting electronic structure is strongly temperature dependent, and at T*≈160 K the system undergoes an insulator-to-metal transition induced by the withdrawal of 4 f electrons from the Fermi volume, the system becoming metallic and nonmagnetic. The G d3 + ESR fine structure coalesces into a single Dysonian resonance, as in metals. Our simulations suggest that exchange narrowing via the usual Korringa mechanism is not enough to describe the thermal behavior of the G d3 + ESR spectra in the entire temperature region (4.2-300 K). We propose that the temperature activated fluctuating valence of the Ce ions is the key ingredient that fully describes this unique temperature dependence of the G d3 + ESR fine structure.

  15. Kondo Destruction in RKKY-Coupled Kondo Lattice and Multi-Impurity Systems

    NASA Astrophysics Data System (ADS)

    Nejati, Ammar; Ballmann, Katinka; Kroha, Johann

    2017-03-01

    In a Kondo lattice, the spin exchange coupling between a local spin and the conduction electrons acquires nonlocal contributions due to conduction electron scattering from surrounding local spins and the subsequent RKKY interaction. It leads to a hitherto unrecognized interference of Kondo screening and the RKKY interaction beyond the Doniach scenario. We develop a renormalization group theory for the RKKY-modified Kondo vertex. The Kondo temperature TK(y ) is suppressed in a universal way, controlled by the dimensionless RKKY coupling parameter y . Complete spin screening ceases to exist beyond a critical RKKY strength yc even in the absence of magnetic ordering. At this breakdown point, TK(y ) remains nonzero and is not defined for larger RKKY couplings y >yc. The results are in quantitative agreement with STM spectroscopy experiments on tunable two-impurity Kondo systems. The possible implications for quantum critical scenarios in heavy-fermion systems are discussed.

  16. Block entropy and quantum phase transition in the anisotropic Kondo necklace model

    NASA Astrophysics Data System (ADS)

    Mendoza-Arenas, J. J.; Franco, R.; Silva-Valencia, J.

    2010-06-01

    We study the von Neumann block entropy in the Kondo necklace model for different anisotropies η in the XY interaction between conduction spins using the density matrix renormalization group method. It was found that the block entropy presents a maximum for each η considered, and, comparing it with the results of the quantum criticality of the model based on the behavior of the energy gap, we observe that the maximum block entropy occurs at the quantum critical point between an antiferromagnetic and a Kondo singlet state, so this measure of entanglement is useful for giving information about where a quantum phase transition occurs in this model. We observe that the block entropy also presents a maximum at the quantum critical points that are obtained when an anisotropy Δ is included in the Kondo exchange between localized and conduction spins; when Δ diminishes for a fixed value of η, the critical point increases, favoring the antiferromagnetic phase.

  17. Frequency Regimes of Kondo Dynamics in a Single-Electron Transistor

    NASA Astrophysics Data System (ADS)

    Hemingway, Bryan; Kogan, Andrei; Herbert, Stephen; Melloch, Michael

    2013-03-01

    It has been theoretically predicted that the Kondo temperature, TK, serves as the intrinsic timescale for the formation of Kondo correlations between conduction electrons and local spin moments. To probe this timescale, we have measured the time averaged differential conductance, =d /dVds, of a single electron transistor in the spin 1/2 Kondo regime in presence of an oscillating bias voltage, V(t)=Vds+VAC sin(2 πft). We present the amplitude dependent conductance over select frequencies spanning several orders of magnitude below TK to twice TK (TK ~ 16GHz). At frequencies above TK, we find good agreement with theory [Kaminski, et al. Phys. Rev. B 62, 8154 (2000)] in both the low (VAC ~ TK/10) and high (VAC ~ 10TK) amplitude regimes. The onset of non-adiabatic conductance behavior occurs well below prediction, f ~ TK, and becomes more apparent as the frequency nears TK. Supported by NSF DMR award Nos. 0804199 and 1206784.

  18. Metallic ferromagnetism in the Kondo lattice

    PubMed Central

    Yamamoto, Seiji J.; Si, Qimiao

    2010-01-01

    Metallic magnetism is both ancient and modern, occurring in such familiar settings as the lodestone in compass needles and the hard drive in computers. Surprisingly, a rigorous theoretical basis for metallic ferromagnetism is still largely missing. The Stoner approach perturbatively treats Coulomb interactions when the latter need to be large, whereas the Nagaoka approach incorporates thermodynamically negligible holes into a half-filled band. Here, we show that the ferromagnetic order of the Kondo lattice is amenable to an asymptotically exact analysis over a range of interaction parameters. In this ferromagnetic phase, the conduction electrons and local moments are strongly coupled but the Fermi surface does not enclose the latter (i.e., it is “small”). Moreover, non-Fermi-liquid behavior appears over a range of frequencies and temperatures. Our results provide the basis to understand some long-standing puzzles in the ferromagnetic heavy fermion metals, and raise the prospect for a new class of ferromagnetic quantum phase transitions. PMID:20798053

  19. Anomalous Behavior of High Quality Factor Planar Superconducting Resonators

    NASA Astrophysics Data System (ADS)

    Megrant, Anthony; Chen, Zijun; Chiaro, Ben; Dunsworth, Andrew; Quintana, Chris; Campbell, Brooks; Kelly, Julian; Barends, Rami; Chen, Yu; Jeffrey, Evan; Mutus, Josh; Neill, Charles; O'Malley, Peter; Sank, Daniel; Vainsencher, Amit; Wenner, Jim; White, Ted; Bochmann, Jorg; Hoi, Iochun; Palmstrom, Christopher; Martinis, John; Cleland, Andrew

    2014-03-01

    Superconducting coplanar waveguide resonators have proven to be invaluable tools in studying some of the decoherence mechanisms found in superconducting qubits. Surface two-level states tend to dominate decoherence at temperatures below Tc/10 and at very low microwave powers, assuming loss through other channels (e.g. quasiparticles, vortices, and radiation loss) has been mitigated through proper shielding and design. I will present recent measurements of resonators whose behavior diverges significantly from the standard two-level state model at low temperatures and low excitation energies, resulting in startling behavior of the internal quality factor. This research was funded by the Office of the Director of National Intelligence (ODNI), Intelligence Advanced Research Projects Activity (IARPA), through the Army Research Office grant W911NF-09-1-0375.

  20. Utilization of localized panel resonant behavior in wind turbine blades.

    SciTech Connect

    Griffith, Daniel Todd

    2010-11-01

    The shear webs and laminates of core panels of wind turbine blades must be designed to avoid panel buckling while minimizing blade weight. Typically, buckling resistance is evaluated by consideration of the load-deflection behavior of a blade using finite element analysis (FEA) or full-scale static loading of a blade to failure under a simulated extreme loading condition. This paper examines an alternative means for evaluating blade buckling resistance using non-destructive modal tests or FEA. In addition, panel resonances can be utilized for structural health monitoring by observing changes in the modal parameters of these panel resonances, which are only active in a portion of the blade that is susceptible to failure. Additionally, panel resonances are considered for updating of panel laminate model parameters by correlation with test data. During blade modal tests conducted at Sandia Labs, a series of panel modes with increasing complexity was observed. This paper reports on the findings of these tests, describes potential ways to utilize panel resonances for blade evaluation, health monitoring, and design, and reports recent numerical results to evaluate panel resonances for use in blade structural health assessment.

  1. Influence of kinetic effects on the resonance behavior of the Multipole Resonance Probe

    NASA Astrophysics Data System (ADS)

    Oberrath, Jens; Mussenbrock, Thomas; Brinkmann, Ralf Peter

    2012-10-01

    Active plasma resonance spectroscopy is a well known diagnostic method. Many concepts of this method are theoretically investigated and realized as a diagnostic tool. One of these tools is the multipole resonance probe (MRP) [1]. The application of such a probe in plasmas with pressures of only a few Pa raises the question whether kinetic effects have to be taken into account or not. To address this question a kinetic model is necessary. A general kinetic model for an electrostatic concept of active plasma resonance spectroscopy has already been presented by the authors [2]. This model can be used to describe the dynamical behavior of the MRP, which is interpretable as a special case of the general model. Neglecting electron-neutral collisions, this model can be solved analytically. Based on this solution we derive an approximated expression for the admittance of the system to investigate the influence of kinetic effects on the resonance behavior of the MRP. [4pt] [1] M. Lapke et al., Plasma Sources Sci. Technol. 20, 2011, 042001[0pt] [2] J. Oberrath et al., Proceedings of the 30th International Conference on Phenomena in Ionized Gases, 28th August - 2nd September, 2011

  2. Kondo bahavior in antiferromagnetic NpPdSn

    NASA Astrophysics Data System (ADS)

    Shrestha, K.; Prokes, K.; Griveau, J.-C.; Jardin, R.; Colineau, E.; Caciuffo, R.; Eloirdi, R.; Gofryk, K.

    Actinide-based intermetallics show a large variety of exotic physical phenomena mainly coming from 5f hybridization with both on-site and neighboring ligand states. Depending on the strength of these process unusual behaviors such as long-range magnetic order, Kondo effect, heavy-fermion ground state, valence fluctuations, and/or superconductivity have been observed. Here we report results of our extensive studies on NpPdSn. The compound crystalizes in hexagonal ZrNiAl-type of crystal structure and is studied by means of x-ray and neutron diffraction, magnetization, heat capacity, electrical resistivity, and thermoelectric power measurements, performed over a wide range of temperatures and applied magnetic fields. All the results revealed Kondo lattice behavior and antiferromagnetic ordering below 19 K. NpPdSn can be classified as a moderately enhanced heavy-fermion system, one of very few known amidst Np-based intermetallics. Work at Idaho National Laboratory was supported by the Department of Energy, Office of Basic Energy Sciences, Materials Sciences, and Engineering Division.

  3. The physics of Kondo impurities in graphene.

    PubMed

    Fritz, Lars; Vojta, Matthias

    2013-03-01

    This article summarizes our understanding of the Kondo effect in graphene, primarily from a theoretical perspective. We shall describe different ways to create magnetic moments in graphene, either by adatom deposition or via defects. For dilute moments, the theoretical description is in terms of effective Anderson or Kondo impurity models coupled to graphene's Dirac electrons. We shall discuss in detail the physics of these models, including their quantum phase transitions and the effect of carrier doping, and confront this with existing experimental data. Finally, we will point out connections to other quantum impurity problems, e.g., in unconventional superconductors, topological insulators, and quantum spin liquids.

  4. Kondo Tunneling through Real and Artificial Molecules

    NASA Astrophysics Data System (ADS)

    Kikoin, Konstantin; Avishai, Yshai

    2001-03-01

    When an asymmetric double dot is hybridized with itinerant electrons, its singlet ground state and lowly excited triplet state cross, leading to a competition between the Zhang-Rice mechanism of singlet-triplet splitting in a confined cluster and the Kondo effect (which accompanies the tunneling through quantum dot under a Coulomb blockade restriction). The rich physics of an underscreened S = 1 Kondo impurity in the presence of low-lying triplet-singlet excitations is exposed and estimates of the magnetic susceptibility and the electric conductance are presented, together with applications for molecule chemisorption on metallic substrates.

  5. Kondo lattice without Nozieres exhaustion effect.

    SciTech Connect

    Kikoin, K.; Kiselev, M. N.; Materials Science Division; Ben-Gurion Univ. of the Negev; Ludwig-Maximilians Univ.

    2006-01-01

    We discuss the properties of layered Anderson/Kondo lattices with metallic electrons confined in 2D xy planes and local spins in insulating layers forming chains in the z direction. Each spin in this model possesses its own 2D Kondo cloud, so that the Nozieres exhaustion problem does not occur. The high-temperature perturbational description is matched to exact low-T Bethe-ansatz solution. The excitation spectrum of the model is gapless both in charge and spin sectors. The disordered phases and possible experimental realizations of the model are briefly discussed.

  6. Kondo tunneling through real and artificial molecules.

    PubMed

    Kikoin, K; Avishai, Y

    2001-03-05

    When an asymmetric double dot is hybridized with itinerant electrons, its singlet ground state and lowly excited triplet state cross, leading to a competition between the Zhang-Rice mechanism of singlet-triplet splitting in a confined cluster and the Kondo effect (which accompanies the tunneling through quantum dot under a Coulomb blockade restriction). The rich physics of an underscreened S = 1 Kondo impurity in the presence of low-lying triplet-singlet excitations is exposed and estimates of the magnetic susceptibility and the electric conductance are presented, together with applications for molecule chemisorption on metallic substrates.

  7. Bohm-Aharonov and Kondo effects on tunneling currents in a mesoscopic ring

    SciTech Connect

    Davidovich, M.A.; Anda, E.V.; Chiappe, G.

    1997-03-01

    We present an analysis of the Kondo effect on the Bohm-Aharonov oscillations of the tunneling currents in a mesoscopic ring with a quantum dot inserted in one of its arms. The system is described by an Anderson-impurity tight-binding Hamiltonian where the electron-electron interaction is restricted to the dot. The currents are obtained using nonequilibrium Green functions calculated through a cumulant diagrammatic expansion in the chain approximation. It is shown that at low temperature, even with the system out of resonance, the Kondo peak provides a channel for the electron to tunnel through the dot, giving rise to the Bohm-Aharonov oscillations of the current. At high temperature these oscillations are important only if the dot level is aligned to the Fermi level, when the resonance condition is satisfied. {copyright} {ital 1997} {ital The American Physical Society}

  8. Effect of anisotropy in the S=1 underscreened Kondo lattice

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simões, Acirete S.; Lacroix, Claudine; Iglesias, José Roberto; Coqblin, Bernard

    2014-12-01

    We study the effect of crystal field anisotropy in the underscreened S=1 Kondo lattice model. Starting from the two orbital Anderson lattice model and including a local anisotropy term, we show, through Schrieffer-Wolff transformation, that local anisotropy is equivalent to an anisotropic Kondo interaction (J∥≠J⊥). The competition and coexistence between ferromagnetism and Kondo effect in this effective model is studied within a generalized mean-field approximation. Several regimes are obtained, depending on the parameters, exhibiting or not coexistence of magnetic order and Kondo effect. Particularly, we show that a re-entrant Kondo phase at low temperature can be obtained. We are also able to describe phases where the Kondo temperature is smaller than the Curie temperature (TKKondo effect and ferromagnetism can be understood within this model.

  9. Two-channel Kondo physics from arsenic bond oscillations in zirconium arsenide selenide

    NASA Astrophysics Data System (ADS)

    Kirchner, Stefan; Cichorek, Tomasz; Bochenek, L.; Schmidt, Marcus; Niewa, Rainer; Czulucki, A.; Auffermann, G.; Steglich, Frank; Kniep, Ruediger

    2015-03-01

    The two-channel Kondo effect is a fascinating but extremely fragile many-body state that has been theoretically discussed extensively. we address metallic compounds of a specific (PbFCl) structure for which a - AT 1 / 2 term to ρ (T) is frequently observed, in line with the two-channel Kondo effect. The origin of this anomalous behavior has remained enigmatic since here, solely the interaction between electrons may account for this behavior, and the two-channel Kondo state is not expected to occur. By combining chemical and structural investigations with various physical property measurements we show that the magnetic field-independent - AT 1 / 2 term to the low-T resistivity observed over two decades in ZrAsxSey with 1.90 <= x + y <= 1.99 originates from vacancies in the layer exclusively built up by As. Furthermore, we can trace back the two-channel Kondo effect in this material to a dynamic Jahn-Teller effect operating at these vacancies. All physical properties of the investigated compounds support this conclusion. Our findings will be relevant also for other metallic systems with pnictogen-pnictogen bondings, e.g., cage-forming compounds like the skutterudites.

  10. Relation between the 0.7 anomaly and the Kondo effect: Geometric crossover between a quantum point contact and a Kondo quantum dot

    NASA Astrophysics Data System (ADS)

    Heyder, Jan; Bauer, Florian; Schubert, Enrico; Borowsky, David; Schuh, Dieter; Wegscheider, Werner; von Delft, Jan; Ludwig, Stefan

    2015-11-01

    Quantum point contacts (QPCs) and quantum dots (QDs), two elementary building blocks of semiconducting nanodevices, both exhibit famously anomalous conductance features: the 0.7 anomaly in the former case, the Kondo effect in the latter. For both the 0.7 anomaly and the Kondo effect, the conductance shows a remarkably similar low-energy dependence on temperature T , source-drain voltage Vsd, and magnetic field B . In a recent publication [F. Bauer et al., Nature (London) 501, 73 (2013), 10.1038/nature12421], we argued that the reason for these similarities is that both a QPC and a Kondo QD (KQD) feature spin fluctuations that are induced by the sample geometry, confined in a small spatial regime, and enhanced by interactions. Here, we further explore this notion experimentally and theoretically by studying the geometric crossover between a QD and a QPC, focusing on the B -field dependence of the conductance. We introduce a one-dimensional model with local interactions that reproduces the essential features of the experiments, including a smooth transition between a KQD and a QPC with 0.7 anomaly. We find that in both cases the anomalously strong negative magnetoconductance goes hand in hand with strongly enhanced local spin fluctuations. Our experimental observations include, in addition to the Kondo effect in a QD and the 0.7 anomaly in a QPC, Fano interference effects in a regime of coexistence between QD and QPC physics, and Fabry-Perot-type resonances on the conductance plateaus of a clean QPC. We argue that Fabry-Perot-type resonances occur generically if the electrostatic potential of the QPC generates a flatter-than-parabolic barrier top.

  11. Transport across two interacting quantum dots: bulk Kondo, Kondo box and molecular regimes

    NASA Astrophysics Data System (ADS)

    Costa Ribeiro, Laercio; Hamad, Ignacio; Chiappe, Guillermo; Victoriano Anda, Enrique

    2014-03-01

    We analyze the transport properties of a double quantum dot device with both dots coupled to perfect conducting leads and to a finite chain of N non-interacting sites connecting both of them. The inter-dot chain strongly influences the transport across the system and the local density of states of the dots. We study the case of small number of sites, so that Kondo box effects are present. For odd N and small coupling between the inter-dot chain and the dots, a state with two coexisting Kondo regimes develops: the bulk Kondo due to the quantum dots connected to leads and the one produced by the screening of the quantum dots spins by the spin in the finite chain. As the coupling to the inter-dot chain increases, there is a crossover to a molecular Kondo effect, due to the screening of the molecule spin by the leads. For even N the two-Kondo temperatures regime does not develop and the physics is dominated by the usual competition between Kondo and antiferromagnetism. We finally study how the transport properties are affected as N is increased. We used exact multi-configurational Lanczos calculations and finite U slave-boson mean-field theory. The results obtained with both methods describe qualitatively and also quantitatively the same physics.

  12. Transport across two interacting quantum dots: Bulk Kondo, Kondo box, and molecular regimes

    NASA Astrophysics Data System (ADS)

    Ribeiro, L. C.; Hamad, I. J.; Chiappe, G.; Anda, E. V.

    2014-01-01

    We analyze the transport properties of a double quantum dot device with both dots coupled to perfect conducting leads and to a finite chain of N noninteracting sites connecting both of them. The interdot chain strongly influences the transport across the system and the local density of states of the dots. We study the case of a small number of sites, so that Kondo box effects are present, varying the coupling between the dots and the chain. For odd N and small coupling between the interdot chain and the dots, a state with two coexisting Kondo regimes develops: the bulk Kondo due to the quantum dots connected to leads and the one produced by the screening of the quantum dot spins by the spin in the finite chain at the Fermi level. As the coupling to the interdot chain increases, there is a crossover to a molecular Kondo effect, due to the screening of the molecule (formed by the finite chain and the quantum dots) spin by the leads. For even N the two Kondo temperatures regime does not develop and the physics is dominated by the usual competition between Kondo and antiferromagnetism between the quantum dots. We finally study how the transport properties are affected as N is increased. For the study we used exact multiconfigurational Lanczos calculations and finite-U slave-boson mean-field theory at T =0. The results obtained with both methods describe qualitatively and also quantitatively the same physics.

  13. Resonant behavior of a fractional oscillator with fluctuating frequency

    NASA Astrophysics Data System (ADS)

    Soika, Erkki; Mankin, Romi; Ainsaar, Ain

    2010-01-01

    The long-time behavior of the first moment for the output signal of a fractional oscillator with fluctuating frequency subjected to an external periodic force is considered. Colored fluctuations of the oscillator eigenfrequency are modeled as a dichotomous noise. The viscoelastic type friction kernel with memory is assumed as a power-law function of time. Using the Shapiro-Loginov formula, exact expressions for the response to an external periodic field and for the complex susceptibility are presented. On the basis of the exact formulas it is demonstrated that interplay of colored noise and memory can generate a variety of cooperation effects, such as multiresonances versus the driving frequency and the friction coefficient as well as stochastic resonance versus noise parameters. The necessary and sufficient conditions for the cooperation effects are also discussed. Particularly, two different critical memory exponents have been found, which mark dynamical transitions in the behavior of the system.

  14. Entanglement in the Anisotropic Kondo Necklace Model

    NASA Astrophysics Data System (ADS)

    Mendoza-Arenas, J. J.; Franco, R.; Silva-Valencia, J.

    We study the entanglement in the one-dimensional Kondo necklace model with exact diagonalization, calculating the concurrence as a function of the Kondo coupling J and an anisotropy η in the interaction between conduction spins, and we review some results previously obtained in the limiting cases η = 0 and 1. We observe that as J increases, localized and conduction spins get more entangled, while neighboring conduction spins diminish their concurrence; localized spins require a minimum concurrence between conduction spins to be entangled. The anisotropy η diminishes the entanglement for neighboring spins when it increases, driving the system to the Ising limit η = 1 where conduction spins are not entangled. We observe that the concurrence does not give information about the quantum phase transition in the anisotropic Kondo necklace model (between a Kondo singlet and an antiferromagnetic state), but calculating the von Neumann block entropy with the density matrix renormalization group in a chain of 100 sites for the Ising limit indicates that this quantity is useful for locating the quantum critical point.

  15. Kondo physics in a dissipative environment

    NASA Astrophysics Data System (ADS)

    Ingersent, K.; Glossop, M. T.; Khoshkhou, N.

    2007-03-01

    In recent years impurity models with quantum critical points have attracted much interest. Well-studied examples include the pseudogap and Bose-Fermi Kondo models. In the former model, the depletion of the host density of states at the Fermi level can destroy the Kondo effect; in the latter case, Kondo screening competes with coupling to a dissipative bosonic bath representing, e.g., collective spin fluctuations of the host. The physics of both models is dominated by an interacting quantum critical point. Here, we focus on the more general case of a magnetic impurity interacting with a pseudogap fermionic density of states ρ(ɛ)|ɛ|^r and with a bosonic bath having a spectral function B(φ)ŝ. Perturbative renormalization-group (RG) studies of the resulting model, discussed in relation to Kondo temperature suppression in underdoped cuprates [1], have established a rich phase diagram with three stable and two critical fixed points. We report nonperturbative results for this model, obtained using a Bose-Fermi numerical RG approach [2]. We discuss the phase diagram for the Ising-anisotropic case, together with quantum critical properties probed via response to a local magnetic field. [1] M. Vojta and M. Kir'can, PRL 90, 157203 (2003). [2] M. T. Glossop and K. Ingersent, PRL 95, 067202 (2005); PRB (2006).

  16. Spatiotemporal behavior and nonlinear dynamics in a phase conjugate resonator

    NASA Technical Reports Server (NTRS)

    Liu, Siuying Raymond

    1993-01-01

    The work described can be divided into two parts. The first part is an investigation of the transient behavior and stability property of a phase conjugate resonator (PCR) below threshold. The second part is an experimental and theoretical study of the PCR's spatiotemporal dynamics above threshold. The time-dependent coupled wave equations for four-wave mixing (FWM) in a photorefractive crystal, with two distinct interaction regions caused by feedback from an ordinary mirror, was used to model the transient dynamics of a PCR below threshold. The conditions for self-oscillation were determined and the solutions were used to define the PCR's transfer function and analyze its stability. Experimental results for the buildup and decay times confirmed qualitatively the predicted behavior. Experiments were carried out above threshold to study the spatiotemporal dynamics of the PCR as a function of Pragg detuning and the resonator's Fresnel number. The existence of optical vortices in the wavefront were identified by optical interferometry. It was possible to describe the transverse dynamics and the spatiotemporal instabilities by modeling the three-dimensional-coupled wave equations in photorefractive FWM using a truncated modal expansion approach.

  17. Spatiotemporal behavior and nonlinear dynamics in a phase conjugate resonator

    NASA Astrophysics Data System (ADS)

    Liu, Siuying Raymond

    1993-12-01

    The work described can be divided into two parts. The first part is an investigation of the transient behavior and stability property of a phase conjugate resonator (PCR) below threshold. The second part is an experimental and theoretical study of the PCR's spatiotemporal dynamics above threshold. The time-dependent coupled wave equations for four-wave mixing (FWM) in a photorefractive crystal, with two distinct interaction regions caused by feedback from an ordinary mirror, was used to model the transient dynamics of a PCR below threshold. The conditions for self-oscillation were determined and the solutions were used to define the PCR's transfer function and analyze its stability. Experimental results for the buildup and decay times confirmed qualitatively the predicted behavior. Experiments were carried out above threshold to study the spatiotemporal dynamics of the PCR as a function of Pragg detuning and the resonator's Fresnel number. The existence of optical vortices in the wavefront were identified by optical interferometry. It was possible to describe the transverse dynamics and the spatiotemporal instabilities by modeling the three-dimensional-coupled wave equations in photorefractive FWM using a truncated modal expansion approach.

  18. Thermoelectric properties of the Kondo insulator FeSb2

    NASA Astrophysics Data System (ADS)

    Figueira, M. S.; Silva-Valencia, J.; Franco, R.

    2012-06-01

    Recently it was shown [A. Bentien, S. Johnsen, G.K.H. Madsen, B.B. Iversen, F. Steglich, Europhys. Lett. 80, 17008 (2007)], that the strongly correlated Kondo insulator FeSb2 exhibits a colossal Seebeck coefficient; however, due to its large lattice thermal conductivity, the dimensionless thermoelectric figure of merit (zT) is only 0.005 at 12 K. This experimental result motivate us to perform a theoretical study of the thermoelectric properties of Kondo insulators, within the framework of the X-boson approach [R. Franco, M.S. Figueira, M.E. Foglio, Phys. Rev. B 66, 045112 (2002)] for the periodic Anderson model. We consider a set of parameters adequate for describing the compound FeSb2, and we calculate the resistivity, the thermoelectric power (Seebeck coefficient), the charge carrier thermal conductance, the thermoelectric factor power (zT), the Wiedemann-Franz law, the specific heat, and the Sommerfeld's γ coefficient. The result of the colossal maximum of the Seebeck coefficient, at low temperatures, has the same order of magnitude as the experimental result [A. Bentien, S. Johnsen, G.K.H. Madsen, B.B. Iversen, F. Steglich, Europhys. Lett. 80, 17008 (2007)]. We also show that those temperature region presents an intermediate valence behavior, characterized by a moderate increase of the Sommerfeld's γ coefficient.

  19. Spin fluctations and heavy fermions in the Kondo lattice

    SciTech Connect

    Khaliullin, G.G.

    1994-09-01

    This paper studies the spectrum of the spin and electronic excitations of the Kondo lattice at low temperatures. To avoid unphysical states, the Mattis {open_quotes}drone{close_quotes}-fermion representation for localized spins is employed. First, the known Fermi liquid properties of a single impurity are examined. The behavior of the correlator between a localized spin and the electron spin density at large distances shows that the effective interaction between electrons on the Fermi level and low-energy localized spin fluctuations scales as {rho}{sup {minus}1}, where {rho} is the band-state density. This fact is developed into a renormalization of the band spectrum in a periodic lattice. If the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between localized spins is much smaller than the Kondo fluctuation frequency {omega}{sub k}, the temperature of the crossover to the single-parameter Fermi liquid mode is determined by {omega}{sub k}. When the RKKY interaction becomes of order {omega}{sub k}, there is a new scale {omega}{sub sf}, the energy of the (antiferromagnetic) paramagnon mode, with {omega}{sub sf}{much_lt}{omega}{sub k}. Here the coherent Fermi liquid regime is realized only below a temperature T{sub coh} of order {omega}{sub sf}, while above T{sub coh} quasiparticle damping exhibits a linear temperature dependence. Finally, the nuclear-spin relaxation rate is calculated. 42 refs.

  20. Competition between Kondo effect and RKKY physics in graphene magnetism

    NASA Astrophysics Data System (ADS)

    Allerdt, A.; Feiguin, A. E.; Das Sarma, S.

    2017-03-01

    The cooperative behavior of quantum impurities on two-dimensional (2D) materials, such as graphene and bilayer graphene, is characterized by a nontrivial competition between screening (Kondo effect) and Ruderman-Kittel-Kasuya-Yosida (RKKY) magnetism. In addition, due to the small density of states at the Fermi level, impurities may not couple to the conduction electrons at all, behaving as free moments. Employing a recently developed exact numerical method to study multi-impurity lattice systems, we obtain nonperturbative results that dramatically depart from expectations based on the conventional RKKY theory. At half filling and for weak coupling, impurities remain in the local moment regime when they are on opposite sublattices, up to a critical value of the interactions when they start coupling antiferromagnetically with correlations that decay very slowly with interimpurity distance. At finite doping, away from half filling, ferromagnetism is completely absent and the physics is dominated by a competition between antiferromagnetism and Kondo effect. In bilayer graphene, impurities on opposite layers behave as free moments, unless the interaction is of the order of the hopping or larger.

  1. Kondo screening in two-dimensional p -type transition-metal dichalcogenides

    NASA Astrophysics Data System (ADS)

    Phillips, Michael; Aji, Vivek

    2017-02-01

    Systems with strong spin-orbit coupling support a number of new phases of matter and novel phenomena. This work focuses on the interplay of spin-orbit coupling and interactions in yielding correlated phenomena in two-dimensional transition-metal dichalcogenides. In particular we explore the physics of Kondo screening resulting from the lack of centrosymmetry, large spin splitting, and spin valley locking in hole-doped systems. The key ingredients are (i) valley-dependent spin-momentum locking perpendicular to the two-dimensional crystal, (ii) a single nondegenerate Fermi surface per valley, and (iii) nontrivial Berry curvature associated with the low-energy bands. The resulting Kondo resonance has a finite-triplet component and nontrivial momentum space structure which facilitates new approaches to both probing and manipulating the correlated state. Using a variational wave function and the numerical renormalization group approaches we study the nature of the Kondo resonance both in the absence and presence of circularly polarized light. The latter induces an imbalance in the population of the two valleys leading to novel magnetic phenomena in the correlated state.

  2. Nonlinear resonant behavior of microbeams over the buckled state

    NASA Astrophysics Data System (ADS)

    Farokhi, Hamed; Ghayesh, Mergen H.; Amabili, Marco

    2013-11-01

    The present study investigates the nonlinear resonant behavior of a microbeam over its buckled (non-trivial) configuration. The system is assumed to be subjected to an axial load along with a distributed transverse harmonic load. The axial load is increased leading the system to lose the stability via a pitchfork bifurcation; the postbuckling configuration is obtained and the nonlinear resonant response of the system over the buckled state is examined. More specifically, the nonlinear equation of motion is obtained employing Hamilton’s principle along with the modified couple stress theory. The continuous system is truncated into a system with finite degrees of freedom; the Galerkin scheme is employed to discretize the nonlinear partial differential equation of motion into a set of ordinary differential equations. This set of equations is solved numerically employing the pseudo-arclength continuation technique; first a nonlinear static analysis is performed upon this set of equations so as to obtain the onset of buckling (supercritical pitchfork bifurcation) and the buckled configuration of the microbeam. The frequency-response and force-response curves of the system are then constructed over the buckled configurations. A comparison is made between the frequency-response curves obtained by means of the modified couple stress and the classical theories. The effect of different system parameters on the frequency-response and force-response curves is also examined.

  3. Vibrational behaviors of multiwalled-carbon-nanotube-based nanomechanical resonators

    NASA Astrophysics Data System (ADS)

    Li, Chunyu; Chou, Tsu-Wei

    2004-01-01

    This letter studies the promising application of carbon nanotubes as nanoresonators. Both single- and double-walled carbon nanotubes are considered and the significant difference in the vibration behavior between them has been identified. The individual tube wall is treated as frame-like structures and simulated by the molecular-structural-mechanics method. The interlayer van der Waals interactions are represented by Lennard-Jones potential and simulated by a nonlinear truss rod model. The results show that fundamental frequencies of double-walled carbon nanotubes are about 10% lower than those of single-walled carbon nanotubes of the same outer diameter. The noncoaxial vibration of double-walled nanotubes begins at the third resonant frequency and does not significantly diminish the value of double-walled nanotubes as high-frequency nanoresonators.

  4. Dynamical symmetries in Kondo tunneling through complex quantum dots.

    PubMed

    Kuzmenko, T; Kikoin, K; Avishai, Y

    2002-10-07

    Kondo tunneling reveals hidden SO(n) dynamical symmetries of evenly occupied quantum dots. As is exemplified for an experimentally realizable triple quantum dot in parallel geometry, the possible values n=3,4,5,7 can be easily tuned by gate voltages. Following construction of the corresponding o(n) algebras, scaling equations are derived and Kondo temperatures are calculated. The symmetry group for a magnetic field induced anisotropic Kondo tunneling is SU(2) or SO(4).

  5. The Kondo effect and coherent transport in stacking-faults-free wurtzite InAs nanowires

    NASA Astrophysics Data System (ADS)

    Kretinin, Andrey V.; Popovitz-Biro, Ronit; Mahalu, Diana; Oreg, Yuval; Heiblum, Moty; Shtrikman, Hadas

    2011-12-01

    The crystalline perfection of wurtzite InAs nanowires grown by the Vapor-Liquid-Solid Molecular Beam Epitaxy technique in combination with careful fabrication of nanowire-based FET devices allowed us to observe a variety of phenomena associated with mesoscopic coherent transport. When the single nanowire channel is nearly pinched-off the Coulomb blockade conductance oscillations exhibit well-pronounced Kondo effect approaching the conductance unitary limit. At some gate voltages the breaking of odd-even parity of the Kondo effect related to the formation of the triplet ground state is observed. At higher gate voltages when the channel is open we observe the Fabry-Pérot type conductance oscillations. The length of the Fabry-Pérot electron resonator deduced from the period of the oscillations is in agreement with the physical length of the nanowire device.

  6. On the zero-bias anomaly and Kondo physics in quantum point contacts near pinch-off.

    PubMed

    Xiang, S; Xiao, S; Fuji, K; Shibuya, K; Endo, T; Yumoto, N; Morimoto, T; Aoki, N; Bird, J P; Ochiai, Y

    2014-03-26

    We investigate the linear and non-linear conductance of quantum point contacts (QPCs), in the region near pinch-off where Kondo physics has previously been connected to the appearance of the 0.7 feature. In studies of seven different QPCs, fabricated in the same high-mobility GaAs/AlGaAs heterojunction, the linear conductance is widely found to show the presence of the 0.7 feature. The differential conductance, on the other hand, does not generally exhibit the zero-bias anomaly (ZBA) that has been proposed to indicate the Kondo effect. Indeed, even in the small subset of QPCs found to exhibit such an anomaly, the linear conductance does not always follow the universal temperature-dependent scaling behavior expected for the Kondo effect. Taken collectively, our observations demonstrate that, unlike the 0.7 feature, the ZBA is not a generic feature of low-temperature QPC conduction. We furthermore conclude that the mere observation of the ZBA alone is insufficient evidence for concluding that Kondo physics is active. While we do not rule out the possibility that the Kondo effect may occur in QPCs, our results appear to indicate that its observation requires a very strict set of conditions to be satisfied. This should be contrasted with the case of the 0.7 feature, which has been apparent since the earliest experimental investigations of QPC transport.

  7. Unexpected observation of spatially separated Kondo scattering and ferromagnetism in Ta alloyed anatase TiO2 thin films

    NASA Astrophysics Data System (ADS)

    Sarkar, T. P.; Gopinadhan, K.; Motapothula, M.; Saha, S.; Huang, Z.; Dhar, S.; Patra, A.; Lu, W. M.; Telesio, F.; Pallecchi, I.; Ariando; Marré, D.; Venkatesan, T.

    2015-08-01

    We report the observation of spatially separated Kondo scattering and ferromagnetism in anatase Ta0.06Ti0.94O2 thin films as a function of thickness (10-200 nm). The Kondo behavior observed in thicker films is suppressed on decreasing thickness and vanishes below ~25 nm. In 200 nm film, transport data could be fitted to a renormalization group theory for Kondo scattering though the carrier density in this system is lower by two orders of magnitude, the magnetic entity concentration is larger by a similar magnitude and there is strong electronic correlation compared to a conventional system such as Cu with magnetic impurities. However, ferromagnetism is observed at all thicknesses with magnetic moment per unit thickness decreasing beyond 10 nm film thickness. The simultaneous presence of Kondo and ferromagnetism is explained by the spatial variation of defects from the interface to surface which results in a dominantly ferromagnetic region closer to substrate-film interface while the Kondo scattering is dominant near the surface and decreasing towards the interface. This material system enables us to study the effect of neighboring presence of two competing magnetic phenomena and the possibility for tuning them.

  8. Magnetic field effects on the DOS of a Kondo quantum dot coupled to LL leads

    NASA Astrophysics Data System (ADS)

    Yang, Kai-Hua; Qin, Chang-Dong; Wang, Huai-Yu; Wang, Xu

    2017-01-01

    We investigate the joint effects of a magnetic field and electron-electron interaction on the tunneling density of states (DOS) of a quantum dot coupled to the Luttinger liquid leads in the Kondo regime. We find that for intralead electron interaction, the DOS develops two peaks deviated from the origin by the Zeeman energy. With the increase of the intralead interaction, a phase transition occurs. For moderately strong interaction, the Zeeman splitting peaks develop into two dips. The splitting of the Kondo peak and dip is not symmetric with respect to up and down spins. In the limit of strong interaction the Zeeman splitting behavior disappears and there appears a power-law scaling behavior.

  9. Thermopower and thermal conductance for a Kondo correlated quantum dot

    NASA Astrophysics Data System (ADS)

    Franco, R.; Silva-Valencia, J.; Figueira, M. S.

    We study the thermopower and thermal conductivity of a gate-defined quantum dot, with a very strong Coulomb repulsion inside the dot, employing the X-boson approach for the impurity Anderson model. Our results show a change in the sign of the thermopower as function of the energy level of the quantum dot (gate voltage), which is associated with an oscillatory behavior and a suppression of the thermopower magnitude at low temperatures. We identify two relevant energy scales: a low temperature scale dominated by the Kondo effect and a T˜Δ temperature scale characterized by charge fluctuations. We also discuss the Wiedemann-Franz relation and the thermoelectric figure of merit. Our results are in qualitative agreement with recent experimental reports and other theoretical treatments.

  10. Quantum Oscillations in Kondo Insulator SmB6

    NASA Astrophysics Data System (ADS)

    Li, Lu

    2015-03-01

    In Kondo insulator samarium hexaboride SmB6, strong correlation and band hybridization lead to a diverging resistance at low temperature. The resistance divergence ends at about 3 Kelvin, a behavior recently demonstrated to arise from the surface conductance. However, questions remain whether and where a topological surface state exists. Quantum oscillations have not been observed to map the Fermi surface. We solve the problem by resolving the Landau Level quantization and Fermi surface topology using torque magnetometry. The observed angular dependence of the Fermi surface cross section suggests two-dimensional surface states on the (101) and (100) plane. Furthermore, similar to the quantum Hall states for graphene, the tracking of the Landau Levels in the infinite magnetic field limit points to -1/2, the Berry phase contribution from the 2D Dirac electronic state.

  11. GW approach to electron-electron interactions within the Anderson impurity model: Kondo correlated quantum transport through two coupled molecules

    NASA Astrophysics Data System (ADS)

    Aksu, H.; Goker, A.

    2017-03-01

    We invoke the nonequilibrium self-consistent GW method within the Anderson impurity model to investigate the dynamical effects occurring in a nanojunction comprised of two coupled molecules. Contrary to the previous single impurity model calculations based on the GW approximation, we observe that the density of states manages to capture both the Kondo resonance and the Breit-Wigner resonances associated with the HOMO and LUMO levels of the molecule. Moreover, the prominence of the Kondo resonance grows dramatically upon switching from the intermediate to the weak coupling regime involving large U / Γ values. The conductance is calculated as a function of the HOMO level and the applied bias across the molecular nanojunction. Calculated conductance curves deviate from the monotonic decay behaviour as a function of the bias when the half-filling condition is not met. The importance of the effect of the molecule-molecule coupling for the electron transport phenomena is also investigated.

  12. Anisotropy induced Kondo splitting in a mechanically stretched molecular junction: A first-principles based study

    SciTech Connect

    Wang, Xiaoli; Hou, Dong; Zheng, Xiao; Yan, YiJing

    2016-01-21

    The magnetic anisotropy and Kondo phenomena in a mechanically stretched magnetic molecular junction are investigated by combining the density functional theory (DFT) and hierarchical equations of motion (HEOM) approach. The system is comprised of a magnetic complex Co(tpy–SH){sub 2} sandwiched between adjacent gold electrodes, which is mechanically stretched in experiments done by Parks et al. [Science 328, 1370 (2010)]. The electronic structure and mechanical property of the stretched system are investigated via the DFT calculations. The HEOM approach is then employed to characterize the Kondo resonance features, based on the Anderson impurity model parameterized from the DFT results. It is confirmed that the ground state prefers the S = 1 local spin state. The structural properties, the magnetic anisotropy, and corresponding Kondo peak splitting in the axial stretching process are systematically evaluated. The results reveal that the strong electron correlations and the local magnetic properties of the molecule magnet are very sensitive to structural distortion. This work demonstrates that the combined DFT+HEOM approach could be useful in understanding and designing mechanically controlled molecular junctions.

  13. Anisotropy induced Kondo splitting in a mechanically stretched molecular junction: A first-principles based study

    NASA Astrophysics Data System (ADS)

    Wang, Xiaoli; Hou, Dong; Zheng, Xiao; Yan, YiJing

    2016-01-01

    The magnetic anisotropy and Kondo phenomena in a mechanically stretched magnetic molecular junction are investigated by combining the density functional theory (DFT) and hierarchical equations of motion (HEOM) approach. The system is comprised of a magnetic complex Co(tpy-SH)2 sandwiched between adjacent gold electrodes, which is mechanically stretched in experiments done by Parks et al. [Science 328, 1370 (2010)]. The electronic structure and mechanical property of the stretched system are investigated via the DFT calculations. The HEOM approach is then employed to characterize the Kondo resonance features, based on the Anderson impurity model parameterized from the DFT results. It is confirmed that the ground state prefers the S = 1 local spin state. The structural properties, the magnetic anisotropy, and corresponding Kondo peak splitting in the axial stretching process are systematically evaluated. The results reveal that the strong electron correlations and the local magnetic properties of the molecule magnet are very sensitive to structural distortion. This work demonstrates that the combined DFT+HEOM approach could be useful in understanding and designing mechanically controlled molecular junctions.

  14. Magnetic-field-induced mixed-level Kondo effect in two-level systems

    SciTech Connect

    Wong, Arturo; Ngo, Anh T.; Ulloa, Sergio E.

    2016-10-17

    We consider a two-orbital impurity system with intra-and interlevel Coulomb repulsion that is coupled to a single conduction channel. This situation can generically occur in multilevel quantum dots or in systems of coupled quantum dots. For finite energy spacing between spin-degenerate orbitals, an in-plane magnetic field drives the system from a local-singlet ground state to a "mixed-level" Kondo regime, where the Zeeman-split levels are degenerate for opposite-spin states. We use the numerical renormalization group approach to fully characterize this mixed-level Kondo state and discuss its properties in terms of the applied Zeeman field, temperature, and system parameters. Under suitable conditions, the total spectral function is shown to develop a Fermi-level resonance, so that the linear conductance of the system peaks at a finite Zeeman field while it decreases as a function of temperature. These features, as well as the local moment and entropy contribution of the impurity system, are commensurate with Kondo physics, which can be studied in suitably tuned quantum dot systems.

  15. Magnetic-field-induced mixed-level Kondo effect in two-level systems

    NASA Astrophysics Data System (ADS)

    Wong, Arturo; Ngo, Anh T.; Ulloa, Sergio E.

    2016-10-01

    We consider a two-orbital impurity system with intra- and interlevel Coulomb repulsion that is coupled to a single conduction channel. This situation can generically occur in multilevel quantum dots or in systems of coupled quantum dots. For finite energy spacing between spin-degenerate orbitals, an in-plane magnetic field drives the system from a local-singlet ground state to a "mixed-level" Kondo regime, where the Zeeman-split levels are degenerate for opposite-spin states. We use the numerical renormalization group approach to fully characterize this mixed-level Kondo state and discuss its properties in terms of the applied Zeeman field, temperature, and system parameters. Under suitable conditions, the total spectral function is shown to develop a Fermi-level resonance, so that the linear conductance of the system peaks at a finite Zeeman field while it decreases as a function of temperature. These features, as well as the local moment and entropy contribution of the impurity system, are commensurate with Kondo physics, which can be studied in suitably tuned quantum dot systems.

  16. Effect of size on the chaotic behavior of nano resonators

    NASA Astrophysics Data System (ADS)

    Alemansour, Hamed; Miandoab, Ehsan Maani; Pishkenari, Hossein Nejat

    2017-03-01

    Present study is devoted to investigate the size effect on chaotic behavior of a micro-electro-mechanical resonator under external electrostatic excitation. Using Galerkin's decomposition method, approximating the actuation force with a new effective lumped model, and neglecting higher order terms in the Taylor-series expansion, a simplified model of the main system is developed. By utilizing the Melnikov's method and based on the new form of the electrostatic force, an expression in terms of the system parameters is developed which can be used to rapidly estimate the chaotic region of the simplified system. Based on the analysis of the simple proposed model, it is shown that the effect of size on chaotic region varies significantly depending on bias voltage. By considering the size effect, it is demonstrated that chaotic vibration initiates at much higher constant voltages than predicted by classical theories; and, in high constant voltages, it is shown that strain gradient theory predicts occurrence of chaos at much lower amplitudes.

  17. Mass-Imbalanced Superconductivity in Effective Two-Channel Kondo Lattice

    NASA Astrophysics Data System (ADS)

    Kusunose, Hiroaki

    2016-11-01

    We propose that mass-imbalanced superconductivity is realized in an effective two-channel Kondo lattice, and its characteristic property appears in electromagnetic responses such as the Meissner effect. Starting from an effective two-channel Kondo lattice model as a low-energy effective theory, and approximating it with two mean-field order parameter components in a self-consistent fashion, it is shown that the balance of the two components is sensitively reflected in the magnitude of the Meissner kernel, while thermodynamic properties are little affected by the balance. This remarkable behavior is understood by the localized character of one partner in the Cooper pair, namely, the effect of the mass imbalance. We briefly mention the relevance to the huge enhancement of the upper critical field under pressure observed in Pr 1-2-20 systems.

  18. Spatiotemporal Behavior and Nonlinear Dynamics in a Phase Conjugate Resonator

    NASA Astrophysics Data System (ADS)

    Liu, Siuying Raymond

    The work described in this dissertation can be divided into two parts. The first part is an investigation of the transient behavior and stability property of a phase conjugate resonator (PCR) below threshold. The second part is an experimental and theoretical study of the PCR's spatiotemporal dynamics above threshold. The time-dependent coupled wave equations for four-wave mixing (FWM) in a photorefractive crystal, with two distinct interaction regions caused by feedback from an ordinary mirror, was used to model the transient dynamics of a PCR below threshold. Analytical expressions of the steady state cavity's fields for the case of nondepleted pumps and an absorption free medium were derived and used to determine the self-oscillation conditions. The solutions, through simple frequency domain transformation techniques, were used to define the PCR's transfer function and analyse its stability. Taking into account pump depletion and medium absorption, the transient buildup and decay times of the cavity's fields as well as the specularly reflected and phase conjugate reflected intensities were numerically calculated as functions of a number of system parameters such as the coupling parameter and the pump and probe ratios. Experiments were carried out above threshold to study the spatiotemporal dynamics of the PCR as a function of the Bragg detuning achieved by misaligning one of the two pump beams and of the degree of transverse confinement controlled by varying the resonator's Fresnel number. The temporal aspects of the beam's complexity were studied by local intensity time series, power spectra, and reconstructed pseudo phase portraits. The transverse dynamics and the spatiotemporal instabilities were also described by modeling the three dimensional coupled wave equations in photorefractive FWM, using a truncated modal expansion approach. Numerical solutions of the model revealed the presence and motion of optical vortices in the wavefront. Simulations using the

  19. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: Anomalous Kondo-Switching Effect of a Spin-Flip Quantum Dot Embedded in an Aharonov-Bohm Ring

    NASA Astrophysics Data System (ADS)

    Chen, Xiong-Wen; Shi, Zhen-Gang; Song, Ke-Hui

    2009-11-01

    We theoretically investigate the Kondo effect of a quantum dot embedded in a mesoscopic Aharonov-Bohm (AB) ring in the presence of the spin flip processes by means of the one-impurity Anderson Hamiltonian. Based on the slave-boson mean-field theory, we find that in this system the persistent current (PC) sensitively depends on the parity and size of the AB ring and can be tuned by the spin-flip scattering (R). In the small AB ring, the PC is suppressed due to the enhancing R weakening the Kondo resonance. On the contrary, in the large AB ring, with R increasing, the peak of PC firstly moves up to max-peak and then down. Especially, the PC phase shift of π appears suddenly with the proper value of R, implying the existence of the anomalous Kondo effect in this system. Thus this system may be a candidate for quantum switch.

  20. Kondo interactions from band reconstruction in YbInCu4

    SciTech Connect

    Jarrige, I.; Kotani, A.; Yamaoka, H.; Tsujii, N.; Ishii, K.; Upton, M.; Casa, D.; Kim, J.; Gog, T.; Hancock, J. N.

    2015-03-27

    We combine resonant inelastic X-ray scattering (RIXS) and model calculations in the Kondo lattice compound YbInCu₄, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T≃42 K. In this study, the bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasi-gap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system.

  1. Kondo physics of the Anderson impurity model by distributional exact diagonalization

    NASA Astrophysics Data System (ADS)

    Motahari, S.; Requist, R.; Jacob, D.

    2016-12-01

    The distributional exact diagonalization (DED) scheme is applied to the description of Kondo physics in the Anderson impurity model. DED maps Anderson's problem of an interacting impurity level coupled to an infinite bath onto an ensemble of finite Anderson models, each of which can be solved by exact diagonalization. An approximation to the self-energy of the original infinite model is then obtained from the ensemble-averaged self-energy. Using Friedel's sum rule, we show that the particle number constraint, a central ingredient of the DED scheme, ultimately imposes Fermi liquid behavior on the ensemble-averaged self-energy, and thus is essential for the description of Kondo physics within DED. Using the numerical renormalization group (NRG) method as a benchmark, we show that DED yields excellent spectra, both inside and outside the Kondo regime for a moderate number of bath sites. Only for very strong correlations (U /Γ ≫10 ) does the number of bath sites needed to achieve good quantitative agreement become too large to be computationally feasible.

  2. Theory of scanning tunneling spectroscopy: from Kondo impurities to heavy fermion materials

    NASA Astrophysics Data System (ADS)

    Morr, Dirk K.

    2017-01-01

    Kondo systems ranging from the single Kondo impurity to heavy fermion materials present us with a plethora of unconventional properties whose theoretical understanding is still one of the major open problems in condensed matter physics. Over the last few years, groundbreaking scanning tunneling spectroscopy (STS) experiments have provided unprecedented new insight into the electronic structure of Kondo systems. Interpreting the results of these experiments—the differential conductance and the quasi-particle interference spectrum—however, has been complicated by the fact that electrons tunneling from the STS tip into the system can tunnel either into the heavy magnetic moment or the light conduction band states. In this article, we briefly review the theoretical progress made in understanding how quantum interference between these two tunneling paths affects the experimental STS results. We show how this theoretical insight has allowed us to interpret the results of STS experiments on a series of heavy fermion materials providing detailed knowledge of their complex electronic structure. It is this knowledge that is a conditio sine qua non for developing a deeper understanding of the fascinating properties exhibited by heavy fermion materials, ranging from unconventional superconductivity to non-Fermi-liquid behavior in the vicinity of quantum critical points.

  3. Natural orbitals renormalization group approach to the two-impurity Kondo critical point

    NASA Astrophysics Data System (ADS)

    He, Rong-Qiang; Dai, Jianhui; Lu, Zhong-Yi

    2015-04-01

    The problem of two magnetic impurities in a normal metal exposes the two opposite tendencies in the formation of a singlet ground state, driven respectively by the single-ion Kondo effect with conduction electrons to screen impurity spins or the Ruderman-Kittel-Kasuya-Yosida interaction between the two impurities to directly form impurity spin singlet. However, whether the competition between these two tendencies can lead to a quantum critical point has been debated over more than two decades. Here, we study this problem by applying the newly proposed natural orbitals renormalization group method to a lattice version of the two-impurity Kondo model with a direct exchange K between the two impurity spins. The method allows for unbiased access to the ground state wave functions and low-lying excitations for sufficiently large system sizes. We demonstrate the existence of a quantum critical point, characterized by the power-law divergence of impurity staggered susceptibility with critical exponent γ =0.60 (1 ) , on the antiferromagnetic side of K when the interimpurity distance R is even lattice spacing, while a crossover behavior is recovered when R is odd lattice spacing. These results have ultimately resolved the long-standing discrepancy between the numerical renormalization group and quantum Monte Carlo studies, confirming a link of this two-impurity Kondo critical point to a hidden particle-hole symmetry predicted by the local Fermi liquid theory.

  4. Theory of scanning tunneling spectroscopy: from Kondo impurities to heavy fermion materials.

    PubMed

    Morr, Dirk K

    2017-01-01

    Kondo systems ranging from the single Kondo impurity to heavy fermion materials present us with a plethora of unconventional properties whose theoretical understanding is still one of the major open problems in condensed matter physics. Over the last few years, groundbreaking scanning tunneling spectroscopy (STS) experiments have provided unprecedented new insight into the electronic structure of Kondo systems. Interpreting the results of these experiments-the differential conductance and the quasi-particle interference spectrum-however, has been complicated by the fact that electrons tunneling from the STS tip into the system can tunnel either into the heavy magnetic moment or the light conduction band states. In this article, we briefly review the theoretical progress made in understanding how quantum interference between these two tunneling paths affects the experimental STS results. We show how this theoretical insight has allowed us to interpret the results of STS experiments on a series of heavy fermion materials providing detailed knowledge of their complex electronic structure. It is this knowledge that is a conditio sine qua non for developing a deeper understanding of the fascinating properties exhibited by heavy fermion materials, ranging from unconventional superconductivity to non-Fermi-liquid behavior in the vicinity of quantum critical points.

  5. On the resonant behavior of laminated accelerating structures

    NASA Astrophysics Data System (ADS)

    Ivanyan, M. I.; Avagyan, V. Sh.; Danielyan, V. A.; Tsakanian, A. V.; Vardanyan, A. S.; Zakaryan, V. S.

    2017-03-01

    The laminated round metallic waveguide is one of the promising options for high frequency single-mode accelerating structures. Under certain conditions the longitudinal impedance of such type structures has a narrow-band resonance that corresponds to slowly propagating synchronous TM01 fundamental mode. In this paper the resonant properties of two parallel plates and rectangular cavity with laminated walls are studied. The first measurement results performed for the copper cavity of rectangular cross section with inner germanium layers at top and bottom walls are presented. The measurements show the existence of a dedicated resonant frequency being in a good agreement with the one predicted for the corresponding laminated parallel plates.

  6. Linear and nonlinear behavior of crystalline optical whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy A.; Matsko, Andrey B.; Ilchenko, Vladimir S.; Maleki, Lute

    2004-01-01

    We demonstrate strong nonlinear behavior of high-Q whispering gallery mode (WGM) resonators made out of various crystals adn devices based on the resonators. The maximum WGM optical Q-fact or achieved at room temperature exceeds 2X10 to the tenth power.

  7. Collective Kondo effect in the Anderson-Hubbard lattice

    NASA Astrophysics Data System (ADS)

    Fazekas, P.; Itai, K.

    1997-02-01

    The periodic Anderson model is extended by switching on a Hubbard U for the conduction electrons. We use the Gutzwiller variational method to study the nearly integral valent limit. The lattice Kondo energy contains the U-dependent chemical potential of the Hubbard subsystem in the exponent, and the correlation-induced band narrowing in the prefactor. Both effects tend to suppress the Kondo scale, which can be understood to result from the blocking of hybridization. At half-filling, we find a Brinkman-Rice-type transition from a Kondo insulator to a Mott insulator.

  8. Pairing correlations near a Kondo-destruction quantum critical point

    NASA Astrophysics Data System (ADS)

    Pixley, J. H.; Deng, Lili; Ingersent, Kevin; Si, Qimiao

    2015-05-01

    Motivated by the unconventional superconductivity observed in heavy-fermion metals, we investigate pairing susceptibilities near a continuous quantum phase transition of the Kondo-destruction type. We solve two-impurity Bose-Fermi Anderson models with Ising and Heisenberg forms of the interimpurity exchange interaction using continuous-time quantum Monte Carlo and numerical renormalization-group methods. Each model exhibits a Kondo-destruction quantum critical point separating Kondo-screened and local-moment phases. For antiferromagnetic interimpurity exchange interactions, singlet pairing is found to be enhanced in the vicinity of the transition. Implications of this result for heavy-fermion superconductivity are discussed.

  9. Nine-year aging behavior of the ceramic flatpack resonator

    SciTech Connect

    Beetley, D.E.

    1990-03-06

    GE has developed a multichannel, high precision aging{asterisk} measurement facility capable of high volume testing of resonators. Features of the facility considered unique for production aging systems test include: (1) Loran-C/disciplined time-frequency (DTF) oscillator frequency standard, (2) direct current power bus design, (3) measurement and switching techniques, and (4) high volume automatic precision resonator aging. Computer-controlled data acquisition is used for unattended operation. Facility requirements included frequency measurement with sufficient precision to allow 20- year extrapolation of resonator frequency shift using 30 data points. The frequency reference is traceable to the National Institute of Standards and Technology (NIST). Long-term extrapolation required selection of a model which would most accurately reflect the major processes involved in aging. In order to verify the accuracy of model extrapolation, a group of resonators has been maintained in test for more than nine years. 9 refs., 16 figs.

  10. Anomalous three-dimensional bulk ac conduction within the Kondo gap of SmB6 single crystals

    NASA Astrophysics Data System (ADS)

    Laurita, N. J.; Morris, C. M.; Koohpayeh, S. M.; Rosa, P. F. S.; Phelan, W. A.; Fisk, Z.; McQueen, T. M.; Armitage, N. P.

    2016-10-01

    The Kondo insulator SmB6 has long been known to display anomalous transport behavior at low temperatures, T <5 K. In this temperatures range, a plateau is observed in the dc resistivity, contrary to the exponential divergence expected for a gapped system. Recent theoretical calculations suggest that SmB6 may be the first topological Kondo insulator (TKI) and propose that the residual conductivity is due to topological surface states which reside within the Kondo gap. Since the TKI prediction many experiments have claimed to observe high mobility surface states within a perfectly insulating hybridization gap. Here, we investigate the low energy optical conductivity within the hybridization gap of single crystals of SmB6 via time domain terahertz spectroscopy. Samples grown by both optical floating zone and aluminum flux methods are investigated to probe for differences originating from sample growth techniques. We find that both samples display significant three-dimensional bulk conduction originating within the Kondo gap. Although SmB6 may be a bulk dc insulator, it shows significant bulk ac conduction that is many orders of magnitude larger than any known impurity band conduction. The nature of these in-gap states and their coupling with the low energy spin excitons of SmB6 is discussed. Additionally, the well-defined conduction path geometry of our optical experiments allows us to show that any surface states, which lie below our detection threshold if present, must have a sheet resistance of R /square≥ 1000 Ω .

  11. Non-Kondo many-body physics in a Majorana-based Kondo type system

    NASA Astrophysics Data System (ADS)

    van Beek, Ian J.; Braunecker, Bernd

    2016-09-01

    We carry out a theoretical analysis of a prototypical Majorana system, which demonstrates the existence of a Majorana-mediated many-body state and an associated intermediate low-energy fixed point. Starting from two Majorana bound states, hosted by a Coulomb-blockaded topological superconductor and each coupled to a separate lead, we derive an effective low-energy Hamiltonian, which displays a Kondo-like character. However, in contrast to the Kondo model which tends to a strong- or weak-coupling limit under renormalization, we show that this effective Hamiltonian scales to an intermediate fixed point, whose existence is contingent upon teleportation via the Majorana modes. We conclude by determining experimental signatures of this fixed point, as well as the exotic many-body state associated with it.

  12. Spin dynamics and Kondo physics in optical tweezers

    NASA Astrophysics Data System (ADS)

    Lin, Yiheng; Lester, Brian J.; Brown, Mark O.; Kaufman, Adam M.; Long, Junling; Ball, Randall J.; Isaev, Leonid; Wall, Michael L.; Rey, Ana Maria; Regal, Cindy A.

    2016-05-01

    We propose to use optical tweezers as a toolset for direct observation of the interplay between quantum statistics, kinetic energy and interactions, and thus implement minimum instances of the Kondo lattice model in systems with few bosonic rubidium atoms. By taking advantage of strong local exchange interactions, our ability to tune the spin-dependent potential shifts between the two wells and complete control over spin and motional degrees of freedom, we design an adiabatic tunneling scheme that efficiently creates a spin-singlet state in one well starting from two initially separated atoms (one atom per tweezer) in opposite spin state. For three atoms in a double-well, two localized in the lowest vibrational mode of each tweezer and one atom in an excited delocalized state, we plan to use similar techniques and observe resonant transfer of two-atom singlet-triplet states between the wells in the regime when the exchange coupling exceeds the mobile atom hopping. Moreover, we argue that such three-atom double-tweezers could potentially be used for quantum computation by encoding logical qubits in collective spin and motional degrees of freedom. Current address: Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.

  13. Fano-Andreev effect in Quantum Dots in Kondo regime

    NASA Astrophysics Data System (ADS)

    Orellana, Pedro; Calle, Ana Maria; Pacheco, Monica; Apel, Victor

    In the present work, we investigate the transport through a T-shaped double quantum dot system coupled to two normal leads and to a superconducting lead. We study the role of the superconducting lead in the quantum interferometric features of the double quantum dot and by means of a slave boson mean field approximation at low temperature regime. We inquire into the influence of intradot interactions in the electronic properties of the system as well. Our results show that Fano resonances due to Andreev bound states are exhibited in the transmission from normal to normal lead as a consequence of quantum interference and proximity effect. This Fano effect produced by Andreev bound states in a side quantum dot was called Fano-Andreev effect, which remains valid even if the electron-electron interaction are taken into account, that is, the Fano-Andreev effect is robust against e-e interactions even in Kondo regime. We acknowledge the financial support from FONDECYT program Grants No. 3140053 and 11400571.

  14. Coexistence of Kondo effect and ferromagnetism in the Underscreened Kondo Lattice model

    NASA Astrophysics Data System (ADS)

    Thomas, C.; Simões, A. S. R.; Iglesias, J. R.; Lacroix, C.; Perkins, N. B.; Coqblin, B.

    2011-12-01

    In this work we use a Schrieffer-Wolff transformation in a two-fold degenerate periodic Anderson lattice to describe the coexistence of Kondo effect and ferromagnetism in some uranium and neptunium compounds. We show that the inclusion of a bandwidth for the f electrons can account for a weak delocalization of 5f electrons. Using a mean field approximation, we show that a maximum of TC versus JK can be found when the bandwidth is proportional to JK.

  15. Kondo Screening and Fermi Surface in the Antiferromagnetic Metal Phase

    NASA Astrophysics Data System (ADS)

    Yamamoto, Seiji; Si, Qimiao

    2006-03-01

    We address the Kondo effect deep inside the antiferromagnetic metal phase of a Kondo lattice Hamiltonian with SU(2) invariance. The local- moment component is described in terms of a non-linear sigma model. The Fermi surface of the conduction electron component is taken to be sufficiently small, so that it is not spanned by the antiferromagnetic wavevector. The effective low energy form of the Kondo coupling simplifies drastically, corresponding to the uniform component of the magnetization that forward-scatters the conduction electrons on their own Fermi surface. We use a combined bosonic and fermionic (Shankar) renormalization group procedure to analyze this effective theory and study the Kondo screening and Fermi surface in the antiferromagnetic phase. The implications for the global magnetic phase diagram, as well as quantum critical points, of heavy fermion metals are discussed.

  16. Frequency behavior of coherent random lasing in diffusive resonant media

    NASA Astrophysics Data System (ADS)

    Tiwari, Anjani Kumar; Uppu, Ravitej; Mujumdar, Sushil

    2012-10-01

    We investigate diffusive propagation of light and consequent random lasing in an amplifying medium comprising resonant spherical scatterers. A Monte-Carlo calculation based on photon propagation via three-dimensional random walks is employed to obtain the dwell-times of light in the system. We compare the inter-scatterer and intra-scatterer dwell-times for representative resonant and non-resonant wavelengths. Our results show that more efficient random lasing, with intense coherent modes, is obtained for a system with intra-scatterer gain. This is also coupled with a larger reduction in frequency fluctuations. We find that such a system can yield almost thresholdless random lasing. Inspired by these results, we discuss a possible practical situation, based on a monodisperse aerosol, wherein frequency controlled coherent random lasing can be obtained. Since our analysis essentially investigates transport of intensity, the results are relevant to coherent random lasers under nonresonant feedback.

  17. Fano resonance in electronic transport through a quantum wire with a side-coupled quantum dot: X-boson treatment

    NASA Astrophysics Data System (ADS)

    Franco, R.; Figueira, M. S.; Anda, E. V.

    2003-04-01

    The transport through a quantum wire with a side-coupled quantum dot is studied. We use the X-boson treatment for the Anderson single impurity model in the limit of U=∞. The conductance presents a minimum for values of T=0 in the crossover from mixed valence to Kondo regime due to a destructive interference between the ballistic channel associated with the quantum wire and the quantum dot channel. We obtain the experimentally studied Fano behavior of the resonance. The conductance as a function of temperature exhibits a logarithmic and universal behavior, that agrees with recent experimental results.

  18. Observation of orbital two-channel Kondo effect in a ferromagnetic L10-MnGa film

    PubMed Central

    Zhu, Lijun; Woltersdorf, Georg; Zhao, Jianhua

    2016-01-01

    The experimental existence and stability of the fixed point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics have been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system resonant scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and a square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, respectively. Our results not only evidence the robust existence of orbital 2CK effect even in the presence of strong magnetic fields and long-range ferromagnetic ordering, but also extend the scope of 2CK host materials from nonmagnetic nanoscale point contacts to diffusive conductors of disordered alloys. PMID:27686323

  19. Observation of orbital two-channel Kondo effect in a ferromagnetic L10-MnGa film

    NASA Astrophysics Data System (ADS)

    Zhu, Lijun; Woltersdorf, Georg; Zhao, Jianhua

    2016-09-01

    The experimental existence and stability of the fixed point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics have been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system resonant scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and a square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, respectively. Our results not only evidence the robust existence of orbital 2CK effect even in the presence of strong magnetic fields and long-range ferromagnetic ordering, but also extend the scope of 2CK host materials from nonmagnetic nanoscale point contacts to diffusive conductors of disordered alloys.

  20. Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2

    PubMed Central

    Aynajian, Pegor; da Silva Neto, Eduardo H.; Parker, Colin V.; Huang, Yingkai; Pasupathy, Abhay; Mydosh, John; Yazdani, Ali

    2010-01-01

    Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu2Si2. We find that, as the temperature is lowered, partial screening of the f electrons’ spins gives rise to a spatially modulated Kondo–Fano resonance that is maximal between the surface U atoms. At T = 17.5 K, URu2Si2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states. PMID:20498090

  1. Gapped excitation in dense Kondo lattice CePtZn

    NASA Astrophysics Data System (ADS)

    Harriger, L.; Disseler, S. M.; Gunasekera, J.; Rodriguez-Rivera, J.; Pixley, J.; Manfrinetti, P.; Dhar, S. K.; Singh, D. K.

    2017-01-01

    We report on neutron scattering and muon spin relaxation measurements of dense Kondo lattice CePtZn. The system develops long-range incommensurate magnetic order as the temperature is reduced below TN=1.75 K. Interestingly, a Q -independent gap at E =0.65 meV in the energy spectrum is found to co-exist with the long-range magnetic order. The gap persists to a very high temperature of T ≃100 K. The Q -independent characteristic and its persistence to high temperature hint that the gapped excitation may be manifesting the excited state of the ground-state doublet of the crystal-field energy levels. However, the observed broadness in the linewidth with distinct temperature and field dependencies makes it a nontrivial phenomenon. Qualitative analysis of the experimental data suggests the possible co-existence of a local critical behavior, which is onset near the critical field of H ≃3 T, with the crystal-field excitation in the dynamic properties.

  2. Spin-Orbit-Coupled Correlated Metal Phase in Kondo Lattices: An Implementation with Alkaline-Earth Atoms

    NASA Astrophysics Data System (ADS)

    Isaev, L.; Schachenmayer, J.; Rey, A. M.

    2016-09-01

    We show that an interplay between quantum effects, strong on-site ferromagnetic exchange interaction, and antiferromagnetic correlations in Kondo lattices can give rise to an exotic spin-orbit coupled metallic state in regimes where classical treatments predict a trivial insulating behavior. This phenomenon can be simulated with ultracold alkaline-earth fermionic atoms subject to a laser-induced magnetic field by observing dynamics of spin-charge excitations in quench experiments.

  3. Extraordinary Hall effect in Kondo-type systems: Contributions from anomalous velocity

    NASA Astrophysics Data System (ADS)

    Levy, P. M.

    1988-10-01

    Kondo systems exhibit a relatively large extraordinary Hall effect which is due to asymmetric resonant scattering of conduction electrons. Theories based on the skew scattering mechanism account for data at high temperatures T>TK (the Kondo temperature) but are unable to explain the very-low-temperature variation of the Hall constant observed in heavy-fermion compounds. Aside from the ordinary Hall effect, caused by the Lorentz force and skew scattering (which makes the scattering probability antisymmetric with respect to interchange of scattering vectors), there exists an additional contribution to the Hall effect known as the anomalous-velocity contribution. This contribution is due to a change in the expression for the current operator in the presence of spin-orbit forces. We derive an expression for the anomalous velocity in terms of the T matrices describing conduction-electron scattering; it is not limited to weak spin-orbit scattering as were previous results. We use the Anderson model of local moments in metals to write this scattering in terms of the mixing interaction between local and conduction electrons, and the local state's Green's function. The transverse Hall current due to anomalous velocity is determined and evaluated in two limits. At high temperature, we use the weak-coupling form of the local state's Green's function; at T=0 K a phase-shift analysis is used, and we rely on the Friedel-Langreth sum rule to give us the phase shift at the Fermi surface. At high temperatures we find that the contribution from anomalous velocity to the Hall constant is quite small compared to that from skew scattering. On the contrary, at low temperatures the anomalous velocity makes the dominant contribution to the Hall constant in Kondo systems.

  4. How does a Kondo impurity respond to its local environment?

    NASA Astrophysics Data System (ADS)

    Heinrich, Andreas

    2008-03-01

    The interplay between localized electrons on a magnetic atom and the conducting electrons in a metal can lead to intriguing many-body ground states such as the Kondo effect. When a spin is Kondo screened by conduction electrons the entire spin system performs a complicated dance that results in the formation of a spin singlet at sufficiently low temperature. For simplicity, most theoretical considerations of Kondo screening focus on magnetic impurities with the lowest possible spin S = 1/2. Such systems can be studied experimentally in exquisite detail and with great control using quantum dots in semiconductor heterostructures or carbon nanotubes. However, in Kondo systems consisting of localized magnetic atoms, the spin is often larger, making the Kondo effect richer and more complex. Here we use the imaging and spectroscopy capabilities of a scanning tunnelling microscope to study how the Kondo screening of a known high-spin atom is determined by its local environment. Co and Ti atoms were deposited on a thin insulating layer (Cu2N) on a copper substrate. We study the influence of external magnetic fields, crystalline magnetic anisotropy, as well as spin-coupling to surrounding atomic spins on the Kondo effect that forms on the Co or Ti atoms. We find that the anisotropy of the crystalline field quenches the high-spin system of Co (S = 3/2) into an effective S = 1/2 Kramers doublet. Surprisingly, much of the impact of these environmental factors on the complex many-body ground state can be understood simply through their effects on the energy levels of the unscreened spin.

  5. Intracavity Beam Behavior in Hybrid Resonator Planar-Waveguide CO(2) Lasers.

    PubMed

    Wasilewski, B; Baker, H J; Hall, D R

    2000-11-20

    We describe a combined computer simulation and experimental investigation of the intracavity spatial beam profile characteristics of a planar-waveguide rf-excited CO(2) laser that incorporates a hybrid waveguide confocal unstable negative-branch resonator. The study includes results for the intracavity lateral beam intensity profile and output power of the laser as a function of resonator mirror misalignment. In addition, the behavior of the unstable resonator, observed experimentally and predicted by the simulation, in generating localized high intensity hot-spots when it is subjected to relatively large misalignment angles is reported.

  6. Majorana modes and Kondo effect in a quantum dot attached to a topological superconducting wire (Presentation Recording)

    NASA Astrophysics Data System (ADS)

    Vernek, Edson; Ruiz-Tijerina, David; da Silva, Luis D.; Egues, José Carlos

    2015-09-01

    Quantum dot attached to topological wires has become an interesting setup to study Majorana bound state in condensed matter[1]. One of the major advantage of using a quantum dot for this purpose is that it provides a suitable manner to study the interplay between Majorana bound states and the Kondo effect. Recently we have shown that a non-interacting quantum dot side-connected to a 1D topological superconductor and to metallic normal leads can sustain a Majorana mode even when the dot is empty. This is due to the Majorana bound state of the wire leaking into the quantum dot. Now we investigate the system for the case in which the quantum dot is interacting[3]. We explore the signatures of a Majorana zero-mode leaking into the quantum dot, using a recursive Green's function approach. We then study the Kondo regime using numerical renormalization group calculations. In this regime, we show that a "0.5" contribution to the conductance appears in system due to the presence of the Majorana mode, and that it persists for a wide range of the dot parameters. In the particle-hole symmetric point, in which the Kondo effect is more robust, the total conductance reaches 3e^2/2h, clearly indicating the coexistence of a Majorana mode and the Kondo resonance in the dot. However, the Kondo effect is suppressed by a gate voltage that detunes the dot from its particle-hole symmetric point as well as by a Zeeman field. The Majorana mode, on the other hand, is almost insensitive to both of them. We show that the zero-bias conductance as a function of the magnetic field follows a well-known universal curve. This can be observed experimentally, and we propose that this universality followed by a persistent conductance of 0.5,e^2/h are evidence for the presence of Majorana-Kondo physics. This work is supported by the Brazilians agencies FAPESP, CNPq and FAPEMIG. [1] A. Y. Kitaev, Ann.Phys. {bf 303}, 2 (2003). [2] E. Vernek, P.H. Penteado, A. C. Seridonio, J. C. Egues, Phys. Rev. B {bf

  7. Influence of two-photon absorption on the dynamic behaviors of microring resonators.

    PubMed

    Li, Qiliang; Chen, Haowen; Xu, Jie; Hu, Miao; Zeng, Ran; Zhou, Xuefang; Li, Shuqin

    2017-04-01

    In this paper, we have investigated the influence of two-photon absorption (TPA) on the dynamic behaviors of all-pass and add-drop microring resonators by using two iterative methods along with the linear stability analysis method. While the incident field is above a certain value, the TPA coefficient has greater influence on the steady state for all-pass and add-drop microring resonators. We use the linear stability analysis method to analyze the stability of the steady state solutions and obtain stability conditions. Results obtained have shown that the change of TPA coefficient will lead to different dynamic behaviors; in addition, while the TPA coefficient is small and its change is slight, the dynamic behaviors of the microring resonators will not change much for most regions. At last, we observe the period windows and route from chaotic to period-N in some original chaotic regions due to the fluctuation of the TPA coefficient.

  8. Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6

    DOE PAGES

    Fuhrman, W. T.; Leiner, Jonathan C.; Nikolić, P.; ...

    2015-01-21

    In this paper, using inelastic neutron scattering, we map a 14 meV coherent resonant mode in the topological Kondo insulator SmB6 and describe its relation to the low energy insulating band structure. The resonant intensity is confined to the X and R high symmetry points, repeating outside the first Brillouin zone and dispersing less than 2 meV, with a 5d-like magnetic form factor. We present a slave-boson treatment of the Anderson Hamiltonian with a third neighbor dominated hybridized band structure. This approach produces a spin exciton below the charge gap with features that are consistent with the observed neutron scattering.more » Finally, we find that maxima in the wave vector dependence of the inelastic neutron scattering indicate band inversion.« less

  9. Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6

    SciTech Connect

    Fuhrman, W. T.; Leiner, Jonathan C.; Nikolić, P.; Granroth, Garrett E.; Stone, Matthew B.; Lumsden, Mark D.; DeBeer-Schmitt, Lisa M.; Alekseev, Pavel A.; Mignot, Jean-Michel; Koohpayeh, S. M.; Cottingham, P.; Phelan, William Adam; Schoop, L.; McQueen, T. M.; Broholm, C.

    2015-01-21

    In this paper, using inelastic neutron scattering, we map a 14 meV coherent resonant mode in the topological Kondo insulator SmB6 and describe its relation to the low energy insulating band structure. The resonant intensity is confined to the X and R high symmetry points, repeating outside the first Brillouin zone and dispersing less than 2 meV, with a 5d-like magnetic form factor. We present a slave-boson treatment of the Anderson Hamiltonian with a third neighbor dominated hybridized band structure. This approach produces a spin exciton below the charge gap with features that are consistent with the observed neutron scattering. Finally, we find that maxima in the wave vector dependence of the inelastic neutron scattering indicate band inversion.

  10. Vibration-mediated Kondo transport in molecular junctions: conductance evolution during mechanical stretching

    PubMed Central

    Rakhmilevitch, David

    2015-01-01

    Summary The vibration-mediated Kondo effect attracted considerable theoretical interest during the last decade. However, due to lack of extensive experimental demonstrations, the fine details of the phenomenon were not addressed. Here, we analyze the evolution of vibration-mediated Kondo effect in molecular junctions during mechanical stretching. The described analysis reveals the different contributions of Kondo and inelastic transport. PMID:26734532

  11. Tuning magnetism by Kondo effect and frustration

    NASA Astrophysics Data System (ADS)

    Löhneysen, Hilbert V.

    2014-03-01

    Heavy-fermion systems are an ideal playground for studying the quantum phase transition (QPT) between paramagnetic and magnetically ordered ground states arising from the competition between Kondo and RKKY interactions. Two different routes have been identified by various experiments, i. e., the more traditional spin-density-wave (SDW) and the Kondo-breakdown approaches. However, up to now an a-priori assignment of a given system to these different routes has not been possible. Yet another route to quantum criticality not included in the above approaches might be geometric frustration of magnetic moments, a route well known for insulating magnets with competing interactions. First experiments on metallic systems have recently been conducted. In the canonical partially frustrated antiferromagnetic system CePd1-xNixAl, the Néel temperature TN(x) decreases, with TN --> 0 at the critical concentration xc ~ 0.144. The low-temperature specific heat C(T) evolves toward C/ Tα ln(T0/ T) for x -->xc. The unusual T dependence of C/ T is compatible with the Hertz-Millis-Moriya (HMM) scenario of quantum criticality if the quantum-critical fluctuations are two-dimensional in nature. Here two-dimensionality might arise from antiferromagnetic planes that are effectively decoupled by the frustrated Ce atoms in between. An exciting possibility is that the planes of frustrated Ce moments form a two-dimensional spin liquid. In the prototypical heavy-fermion system CeCu6-xAux the experiments by Schröder et al. provided the initial evidence of local quantum criticality. While concentration and pressure tuning of the quantum phase transition (QPT) are described by this scenario, magnetic-field tuning the QPT is in line with the SDW scenario. Elastic neutron scattering experiments on CeCu5.5Au0.5 under hydrostatic pressure p show that at p = 8 kbar, TN and the magnetic propagation vector attain almost the values of CeCu5.7Au0.3. This x - p analogy away from the QPT is highly remarkable

  12. Collective behavior of quantum resonators coupled to a metamaterial

    NASA Astrophysics Data System (ADS)

    Felbacq, Didier; Rousseau, Emmanuel

    2016-09-01

    We study a device that consist of quantum resonators coupled to a mesoscopic photonic structure, such as a metasurface or a 2D metamaterial. For metasurfaces, we use surface Bloch modes in order to reach various coupling regimes between the metasurface and a quantum emitter, modelized semi-classically by an oscillator. Using multiple scattering theory and complex plane techniques, we show that the coupling can be characterized by means of a pole-and-zero structure. The regime of strong coupling is shown to be reached when the pole-and- zero pair is broken. For 2D metamaterial, we show the possibility of controlling optically the opening or closing of a gap.

  13. Microwave memristive behavior in split-ring resonator metamaterials

    NASA Astrophysics Data System (ADS)

    Wu, H. Y.; Shi, S. K.; Wang, C. H.; Jiang, X. J.; Yu, G.; Qin, G. Q.; Fu, H.; Zhou, J.

    2016-07-01

    Photonic memristors, which behave as memristors operating with electromagnetic fields, present an effective means to achieve all-optical networking, and can promote the development of optical communications and computer technology. In this paper, we report a microwave memristive phenomenon at room temperature in metamaterials consisting of negative temperature coefficient thermistor ceramic disk and split-ring resonator (SRR). Hysteretic transmission-incident field power loops, the area of which varies with the scan rate of power, (similar to the fingerprint of memristors) were observed in the metamaterials. These effects are attributed to the increasing conductivity of the ceramic disk with increasing temperature generated by the interaction between electromagnetic waves and metamaterials. This work offers new opportunities for the development of photonic memristors.

  14. Pattern of adsorption isotherms in Ono-Kondo coordinates.

    PubMed

    Sumanatrakul, Panita; Abaza, Sarah; Aranovich, Gregory L; Sangwichien, Chayanoot; Donohue, Marc D

    2012-02-15

    The Ono-Kondo lattice density functional theory is used to analyze adsorbate-adsorbate interactions for supercritical systems. In prior work, this approach has been used to study intermolecular interactions in subcritical adsorbed phases, and this has included the study of adsorbate-adsorbate repulsions in the regime of adsorption compression. In this paper, we present the general pattern of adsorption isotherms in Ono-Kondo coordinates; this has not been done in the past. For this purpose, experimental isotherms for adsorption of supercritical fluids (including nitrogen, methane, and carbon dioxide) are plotted in Ono-Kondo coordinates. In addition, we performed Grand Canonical Monte Carlo simulations of adsorption for Lennard-Jones molecules and plotted isotherms in Ono-Kondo coordinates. Our results indicate a pattern of isotherms with regimes of adsorbate-adsorbate attractions at low surface coverage and adsorbate-adsorbate repulsions at high surface coverage. When the generalized Ono-Kondo model is used over a wide range of pressures - from low pressures of the Henry's law regime to supercritical pressures - the slope of the isotherm varies from positive at low pressures to negative at high pressures. The linear sections of these graphs show when the adsorbate-adsorbate interaction energies are approximately constant. When these linear sections have negative slopes, it indicates that the system is in a state of adsorption compression.

  15. Entanglement entropy near Kondo-destruction quantum critical points

    NASA Astrophysics Data System (ADS)

    Pixley, J. H.; Chowdhury, Tathagata; Miecnikowski, M. T.; Stephens, Jaimie; Wagner, Christopher; Ingersent, Kevin

    2015-06-01

    We study the impurity entanglement entropy Se in quantum impurity models that feature a Kondo-destruction quantum critical point (QCP) arising from a pseudogap in the conduction-band density of states or from coupling to a bosonic bath. On the local-moment (Kondo-destroyed) side of the QCP, the entanglement entropy contains a critical component that can be related to the order parameter characterizing the quantum phase transition. In Kondo models describing a spin-Simp,Se assumes its maximal value of ln(2 Simp+1 ) at the QCP and throughout the Kondo phase, independent of features such as particle-hole symmetry and under- or overscreening. In Anderson models, Se is nonuniversal at the QCP and, at particle-hole symmetry, rises monotonically on passage from the local-moment phase to the Kondo phase; breaking this symmetry can lead to a cusp peak in Se due to a divergent charge susceptibility at the QCP. Implications of these results for quantum critical systems and quantum dots are discussed.

  16. Spin-valley Kondo effect in silicon quantum dots

    NASA Astrophysics Data System (ADS)

    Shiau, Shiue Yuan

    Recent progress in the fabrication of silicon-based quantum dots opens the prospect of observing the Kondo effect associated with the valley degree of freedom. We compute the dot density of states using an Anderson impurity model, whose structure mimics the nonlinear conductance through a dot. The density of states is obtained as a function of temperature and applied magnetic field in the Kondo regime using an equation-of-motion approach. We show that there is a very complex peak structure near the Fermi energy in the N =1,2,3 Coulomb blockade regimes, but not in the N =4, with several signatures that distinguish this spin-valley Kondo effect from the usual spin Kondo effect seen in GaAs dots. We also show that the valley index is generally not conserved when electrons tunnel into a silicon dot, though the extent of this non-conservation is expected to be sample-dependent. This valley index non-conservation can be detected in principle from the valley Kondo effect. We identify features of the conductance that should enable experimenters to understand the interplay of Zeeman splitting and valley splitting, as well as the dependence of tunneling on the valley degree of freedom.

  17. Fine structure of the spectra of the Kondo lattice model: Two-site cellular dynamical mean-field theory study

    NASA Astrophysics Data System (ADS)

    Osolin, Žiga; Žitko, Rok

    2017-01-01

    We study the antiferromagnetic and paramagnetic Kondo insulator phases of the Kondo lattice model on the cubic lattice at half filling using the cellular dynamical mean-field theory (CDMFT) with the numerical renormalization group (NRG) as the impurity solver, focusing on the fine details of the spectral function and self-energy. We find that the nonlocal correlations increase the gap in both the antiferromagnetic and Kondo insulator phases and shrink the extent of the antiferromagnetic phase in the phase diagram but do not alter any properties qualitatively. The agreement between the numerical CDMFT results and those within a simple hybridization picture, which adequately describes the overall band structure of the system but neglects all effects on the inelastic-scattering processes, is similar to that of the single-site DMFT results; there are deviations that are responsible for the additional fine structure, in particular for the asymmetric spectral resonances or dips that become more pronounced in the strong-coupling regime close to the antiferromagnet-paramagnetic quantum phase transition. These features appear broader in the CDMFT mostly due to numerical artifacts linked to more aggressive state truncation required in the NRG.

  18. Fridel sum rules for one- and two-channel Kondo models and unitarity paradox via bosonization-refermionization approach

    NASA Astrophysics Data System (ADS)

    Kharitonov, Maxim; Andrei, Natan; Coleman, Piers

    2013-03-01

    We calculate the single-particle Green's functions and scattering amplitudes of the one-channel and channel-anisotropic two-channel Kondo models at the Toulouse and Emery-Kivelson lines, respectively, where exact solutions via the bosonization-refermionization approach are admitted. We demonstrate that in this approach the Friedel sum rules - the relations between the trapped spin and ``flavor'' moments and the scattering phase shifts in the Fermi-liquid regime - arise naturally and elucidate on their subtleties. We also recover the ``unitarity paradox'' - the vanishing of the single-particle scattering amplitude at the channel-symmetric point of the two-channel Kondo model - stemming from non-Fermi-liquid behavior. We discuss the implications of these results for the development of composite pairing in heavy fermion systems. This work was supported by National Science Foundation grants DMR 0907179 (MK, PC) and DMR 1006684 (NA).

  19. Self-other resonance, its control and prosocial inclinations: Brain-behavior relationships.

    PubMed

    Christov-Moore, Leonardo; Iacoboni, Marco

    2016-04-01

    Humans seem to place a positive reward value on prosocial behavior. Evidence suggests that this prosocial inclination is driven by our reflexive tendency to share in the observed sensations, emotions and behavior of others, or "self-other resonance". In this study, we examine how neural correlates of self-other resonance relate to prosocial decision-making. Subjects performed two tasks while undergoing fMRI: observation of a human hand pierced by a needle, and observation and imitation of emotional facial expressions. Outside the scanner, subjects played the Dictator Game with players of low or high income (represented by neutral-expression headshots). Subjects' offers in the Dictator Game were correlated with activity in neural systems associated with self-other resonance and anticorrelated with activity in systems implicated in the control of pain, affect, and imitation. Functional connectivity between areas involved in self-other resonance and top-down control was negatively correlated with subjects' offers. This study suggests that the interaction between self-other resonance and top-down control processes are an important component of prosocial inclinations towards others, even when biological stimuli associated with self-other resonance are limited. These findings support a view of prosocial decision-making grounded in embodied cognition.

  20. Resonant-state expansions and the long-time behavior of quantum decay

    SciTech Connect

    Garcia-Calderon, Gaston; Maldonado, Irene; Villavicencio, Jorge

    2007-07-15

    It is shown that a representation of the decaying wave function as a resonant sum plus a nonexponential integral term may be written as a purely discrete resonant sum by evaluating at long times the integral term by the steepest descents method, and then expanding the resulting expression in terms of resonant states. This leads to a representation that is valid along the exponential and the inverse power in time regimes. A model calculation using the {delta} potential allows us to make a comparison of the expansion with numerical integrations in terms of continuum wave functions and, in the long time regime, with an exact analytic expression of the integral term obtained using the steepest descents method. The results demonstrate that resonant states give a correct description of the long-time behavior of decay.

  1. Modulating resonance behaviors by noise recycling in bistable systems with time delay.

    PubMed

    Sun, Zhongkui; Yang, Xiaoli; Xiao, Yuzhu; Xu, Wei

    2014-06-01

    In this paper, the impact of noise recycling on resonance behaviors is studied theoretically and numerically in a prototypical bistable system with delayed feedback. According to the interior cooperating and interacting activity of noise recycling, a theory has been proposed by reducing the non-Markovian problem into a two-state model, wherein both the master equation and the transition rates depend on not only the current state but also the earlier two states due to the recycling lag and the feedback delay. By virtue of this theory, the formulae of the power spectrum density and the linear response function have been found analytically. And the theoretical results are well verified by numerical simulations. It has been demonstrated that both the recycling lag and the feedback delay play a crucial role in the resonance behaviors. In addition, the results also suggest an alternative scheme to modulate or control the coherence or stochastic resonance in bistable systems with time delay.

  2. Modulating resonance behaviors by noise recycling in bistable systems with time delay

    SciTech Connect

    Sun, Zhongkui Xu, Wei; Yang, Xiaoli; Xiao, Yuzhu

    2014-06-01

    In this paper, the impact of noise recycling on resonance behaviors is studied theoretically and numerically in a prototypical bistable system with delayed feedback. According to the interior cooperating and interacting activity of noise recycling, a theory has been proposed by reducing the non-Markovian problem into a two-state model, wherein both the master equation and the transition rates depend on not only the current state but also the earlier two states due to the recycling lag and the feedback delay. By virtue of this theory, the formulae of the power spectrum density and the linear response function have been found analytically. And the theoretical results are well verified by numerical simulations. It has been demonstrated that both the recycling lag and the feedback delay play a crucial role in the resonance behaviors. In addition, the results also suggest an alternative scheme to modulate or control the coherence or stochastic resonance in bistable systems with time delay.

  3. Kondo screening and beyond: An x-ray absorption and dichroism study of CePt5/Pt(111 )

    NASA Astrophysics Data System (ADS)

    Praetorius, C.; Fauth, K.

    2017-03-01

    We use x-ray absorption spectroscopy as well as its linear and circular magnetic dichroisms to characterize relevant interactions and energy scales in the surface intermetallic CePt5/Pt(111 ). The experiments provide insight into crystal field splitting, effective paramagnetic moments, their Kondo screening and mutual interactions, and thus into many aspects which typically determine the low-temperature behavior of correlated rare-earth compounds. Exploiting the tunability of Ce valence through the thickness-dependent epitaxial strain at the CePt5/Pt(111 ) interface, we are able to systematically investigate the impact of hybridization strength on these interactions. Considerable Kondo screening is indeed observed at all CePt5 thicknesses, and found to be strongest in case of strongest hybridization. While the magnetic response is commensurate with an impurity Kondo scale of TK≳102 K for specimen temperatures T ≳30 K, this is no longer the case at lower temperature. Its detailed study by x-ray circular magnetic dichroism (XMCD) at one specific thickness of CePt5 reveals an anomaly of the susceptibility at T*≈25 K instead, which we tentatively associate with the onset of lattice coherence. At lowest temperature we observe paramagnetic saturation with a small Ce 4 f saturation magnetization. Within the framework of itinerant 4 f electrons, saturation is due to a field-induced Lifshitz transition involving a very heavy band with correspondingly small degeneracy temperature of TF≈7 K. This small energy scale results in the persistence of Curie-Weiss behavior across the entire range of experimentally accessible temperatures (T ≳2 K). Our work highlights the potential of magnetic circular dichroism studies in particular for Kondo and heavy-fermion materials, which so far has remained largely unexplored.

  4. Thermoelectric response of a correlated impurity in the nonequilibrium Kondo regime

    NASA Astrophysics Data System (ADS)

    Dorda, Antonius; Ganahl, Martin; Andergassen, Sabine; von der Linden, Wolfgang; Arrigoni, Enrico

    2016-12-01

    We study nonequilibrium thermoelectric transport properties of a correlated impurity connected to two leads for temperatures below the Kondo scale. At finite bias, for which a current flows across the leads, we investigate the differential response of the current to a temperature gradient. In particular, we compare the influence of a bias voltage and of a finite temperature on this thermoelectric response. This is of interest from a fundamental point of view to better understand the two different decoherence mechanisms produced by a bias voltage and by temperature. Our results show that in this respect the thermoelectric response behaves differently from the electric conductance. In particular, while the latter displays a similar qualitative behavior as a function of voltage and temperature, both in theoretical and experimental investigations, qualitative differences occur in the case of the thermoelectric response. In order to understand this effect, we analyze the different contributions in connection to the behavior of the impurity spectral function versus temperature. Especially in the regime of strong interactions and large enough bias voltages, we obtain a simple picture based on the asymmetric suppression or enhancement of the split Kondo peaks as a function of the temperature gradient. Besides the academic interest, these studies could additionally provide valuable information to assess the applicability of quantum dot devices as responsive nanoscale temperature sensors.

  5. Effective Kondo Model for a Trimer on a Metallic Surface

    NASA Astrophysics Data System (ADS)

    Aligia, A. A.

    2006-03-01

    I consider a Hubbard-Anderson model which describes localized orbitals in three different atoms hybridized both among themselves and with a continuum of extended states. Using a generalized Schrieffer-Wolf transformation, I derive an effective Kondo model for the interaction between the doublet ground state of the isolated trimer and the extended states. For an isoceles trimer with distances a, l, l between the atoms, the Kondo temperature is very small for la when a is small. The results agree with experiments for a Cr trimer on Au(111).

  6. Inelastic transport through Aharonov-Bohm interferometer in Kondo regime

    SciTech Connect

    Yoshii, Ryosuke; Eto, Mikio; Sakano, Rui; Affleck, Ian

    2013-12-04

    We formulate elastic and inelastic parts of linear conductance through an Aharonov-Bohm (AB) ring with an embedded quantum dot in the Kondo regime. The inelastic part G{sub inel} is proportional to T{sup 2} when the temperature T is much smaller than the Kondo temperature T{sub K}, whereas it is negligibly small compared with elastic part G{sub el} when T ≫ T{sub K}. G{sub inel} weakly depends on the magnetic flux penetrating the AB ring, which disturbs the precise detection of G{sub el}/(G{sub el}+G{sub inel}) by the visibility of AB oscillation.

  7. Quadrupolar Kondo effect in uranium heavy-electron materials?

    NASA Technical Reports Server (NTRS)

    Cox, D. L.

    1987-01-01

    The possibility of an electric quadrupole Kondo effect for a non-Kramers doublet on a uranium (U) ion is a cubic metallic host is demonstrated by model calculations showing a Kondo upturn in the resistivity, universal quenching of the quadrupolar moment, and a heavy-electron anomaly in the electronic specific heat. With inclusion of excited crystal-field levels, some of the unusual magnetic-response data in the heavy-electron superconductor UBe13 may be understood. Structural phase transitions at unprecedented low temperatures may occur in U-based heavy-electron materials.

  8. Detecting the Kondo screening cloud around a quantum dot.

    PubMed

    Affleck, I; Simon, P

    2001-03-26

    A fundamental prediction of scaling theories of the Kondo effect is the screening of an impurity spin by a cloud of electrons spread out over a mesoscopic distance. This cloud has never been observed experimentally. Recently, aspects of the Kondo effect have been observed in experiments on quantum dots embedded in quantum wires. Since the length of the wire may be of order the size of the screening cloud, such systems provide an ideal opportunity to observe it. We point out that persistent current measurements in a closed ring provide a conceptually simple way of detecting this fundamental length scale.

  9. Pressure effects on the dissipative behavior of nanocrystalline diamond microelectromechanical resonators

    NASA Astrophysics Data System (ADS)

    Santos, J. T.; Holz, T.; Fernandes, A. J. S.; Costa, F. M.; Chu, V.; Conde, J. P.

    2015-02-01

    Diamond-based microelectromechanical resonators have the potential of enhanced performance due to the chemical inertness of the diamond structural layer and its high Young’s modulus, high wear resistance, low thermal expansion coefficient, and very high thermal conductivity. In this work, the resonance frequency and quality factor of MEMS resonators based on nanocrystalline diamond films are characterized under different air pressures. The dynamic behavior of 50-300 μm long linear bridges and double ended tuning forks, with resonance frequencies between 0.5 and 15 MHz and quality factors as high as 50 000 are described as a function of measurement pressure from high vacuum(~10 mTorr) up to atmospheric conditions. The resonance frequencies and quality factors in vacuum show good agreement with the theoretical models including anchor and thermoelastic dissipation (TED). The Young’s moduli for nanocrystalline diamond films extrapolated from experimental data are between 840-920 GPa. The critical pressure values, at which the quality factor starts decreasing due to dissipation in air, are dependent on the resonator length. Longer structures, with quality factors limited by TED and lower resonance frequencies, have low critical pressures, of the order of 1-10 Torr and go from an intrinsic dissipation, to a molecular dissipation regime and finally to a region of viscous dissipation. Shorter resonators, with higher resonance frequencies and quality factors limited by anchor losses, have higher critical pressures, some higher than atmospheric pressure, and enter directly into the viscous dissipation regime from the intrinsic region.

  10. Thermal oscillatory behavior analysis and dynamic modulation of refractive index in microspherical resonator.

    PubMed

    Wang, Quanlong; Wang, Yue; Guo, Zhen; Wu, Junfeng; Wu, Yihui

    2015-04-01

    The thermal nonlinear effects in whispering-gallery-mode resonators are characterized by oscillatory behavior in the transmission spectrum. Although the thermal linewidth broadening is proven to be practical in mode-locking and dynamic control of the optical path, the oscillatory behavior always leads to instability of mode-locking and influences the control accuracy. We theoretically and experimentally illustrate the thermal oscillatory behavior using a model that combines slow and fast thermal relaxation processes of the microsphere and fluctuations of the pump wavelength. We also report dynamic modulation of the refractive index based on the fast thermal relaxation process.

  11. Mean Motion Resonances in Exoplanet Systems: An Investigation into Nodding Behavior

    NASA Astrophysics Data System (ADS)

    Ketchum, Jacob A.; Adams, Fred C.; Bloch, Anthony M.

    2013-01-01

    Motivated by the large number of extrasolar planetary systems that are near mean motion resonances, this paper explores a related type of dynamical behavior known as "nodding." Here, the resonance angle of a planetary system executes libration (oscillatory motion) for several cycles, circulates for one or more cycles, and then enters once again into libration. This type of complicated dynamics can affect our interpretation of observed planetary systems that are in or near mean motion resonance. This work shows that planetary systems in (near) mean motion resonance can exhibit nodding behavior, and outlines the portion of parameter space where it occurs. This problem is addressed using both full numerical integrations of the planetary systems and via model equations obtained through expansions of the disturbing function. In the latter approach, we identify the relevant terms that allow for nodding. The two approaches are in agreement, and show that nodding often occurs when a small body is in an external mean motion resonance with a larger planet. As a result, the nodding phenomenon can be important for interpreting observations of transit timing variations, where the existence of smaller bodies is inferred through their effects on larger, observed transiting planets. For example, in actively nodding planetary systems, both the amplitude and frequency of the transit timing variations depend on the observational time window.

  12. Self-Other Resonance, Its Control and Prosocial Inclinations: Brain-Behavior Relationships

    PubMed Central

    Christov-Moore, Leonardo; Iacoboni, Marco

    2016-01-01

    Humans seem to place a positive reward value on prosocial behavior. Evidence suggests that this prosocial inclination is driven by our reflexive tendency to share in the observed sensations, emotions and behavior of others, or “self-other resonance”. In this study, we examine how neural correlates of self-other resonance relate to prosocial decision-making. Subjects performed two tasks while undergoing fMRI: Observation of a human hand pierced by a needle, and observation and imitation of emotional facial expressions. Outside the scanner, subjects played the Dictator Game with players of low or high income (represented by neutral-expression headshots). Subjects’ offers in the Dictator Game were correlated with activity in neural systems associated with self-other resonance and anticorrelated with activity in systems implicated in the control of pain, affect and imitation. Activity in these latter systems was specifically correlated with subjects’ diminished sharing towards players of high incomes. Functional connectivity between areas involved in self-other resonance and top-down control was negatively correlated with subjects’ offers. This study suggests that the interaction between self-other resonance and top-down control processes are an important component of prosocial inclinations towards others, even when biological stimuli associated with self-other resonance are limited. These findings support a view of prosocial decision-making that is grounded in embodied cognition. PMID:26954937

  13. MEAN MOTION RESONANCES IN EXOPLANET SYSTEMS: AN INVESTIGATION INTO NODDING BEHAVIOR

    SciTech Connect

    Ketchum, Jacob A.; Adams, Fred C.; Bloch, Anthony M.

    2013-01-10

    Motivated by the large number of extrasolar planetary systems that are near mean motion resonances, this paper explores a related type of dynamical behavior known as 'nodding'. Here, the resonance angle of a planetary system executes libration (oscillatory motion) for several cycles, circulates for one or more cycles, and then enters once again into libration. This type of complicated dynamics can affect our interpretation of observed planetary systems that are in or near mean motion resonance. This work shows that planetary systems in (near) mean motion resonance can exhibit nodding behavior, and outlines the portion of parameter space where it occurs. This problem is addressed using both full numerical integrations of the planetary systems and via model equations obtained through expansions of the disturbing function. In the latter approach, we identify the relevant terms that allow for nodding. The two approaches are in agreement, and show that nodding often occurs when a small body is in an external mean motion resonance with a larger planet. As a result, the nodding phenomenon can be important for interpreting observations of transit timing variations, where the existence of smaller bodies is inferred through their effects on larger, observed transiting planets. For example, in actively nodding planetary systems, both the amplitude and frequency of the transit timing variations depend on the observational time window.

  14. Constructive influence of the induced electron pairing on the Kondo state

    PubMed Central

    Domański, T.; Weymann, I.; Barańska, M.; Górski, G.

    2016-01-01

    Superconducting order and magnetic impurities are usually detrimental to each other. We show, however, that in nanoscopic objects the induced electron pairing can have constructive influence on the Kondo effect originating from the effective screening interactions. Such situation is possible at low temperatures in the quantum dots placed between the conducting and superconducting reservoirs, where the proximity induced electron pairing cooperates with the correlations amplifying the spin-exchange potential. The emerging Abrikosov-Suhl resonance, which is observable in the Andreev conductance, can be significantly enhanced by increasing the coupling to superconducting lead. We explain this intriguing tendency within the Anderson impurity model using: the generalized Schrieffer-Wolff canonical transformation, the second order perturbative treatment of the Coulomb repulsion, and the nonperturbative numerical renormalization group calculations. We also provide hints for experimental observability of this phenomenon. PMID:27009681

  15. Phase diagram of the Kondo necklace model with planar and local anisotropies

    NASA Astrophysics Data System (ADS)

    Mendoza-Arenas, J. J.; Franco, R.; Silva-Valencia, J.

    2010-12-01

    We use the density matrix renormalization group to study the quantum critical behavior of a one-dimensional Kondo necklace model with two anisotropies: η in the XY interaction of conduction spins and Δ in the local exchange between localized and conduction spins (characterized by J). To do so, we calculate the gap between the ground and the first excited state for different values of η and Δ as a function of J, and fit it to a Kosterlitz-Thouless tendency; the point in which the gap vanishes is the quantum critical point Jc. To support our results, we calculate correlation functions and structure factors near the obtained critical points. The use of entanglement measures, specifically the von Neumann block entropy, to identify the quantum phase transition is also presented. Then we build the phase diagram of the model: for every Δ considered, any value of η > 0 generates a quantum phase transition from a Kondo singlet to an antiferromagnetic state at a finite value of J, and as η diminishes, so does Jc; when Δ diminishes for a fixed η, Jc increases, favoring the antiferromagnetic state.

  16. Is the black phase of SmS a topological Kondo insulator?

    NASA Astrophysics Data System (ADS)

    Bauer, Eric; Ghimire, N. J.; Ronning, F.; Batista, C.; Byler, D.; Thompson, J. D.; Rahmanisisan, A.; Fisk, Z.

    2015-03-01

    SmS is a prototypical Kondo insulator where electronic correlations drive a system insulating that would otherwise be metallic. Whether or not such a system is also a topological insulator that hosts a protected metallic surface state, depends on the parity of the wavefunction of the occupied states. However, unlike weakly correlated materials, it is unclear whether state-of-the-art electronic structure calculations accurately predict the parity of the occupied wavefunctions of correlated insulators. Nevertheless, Dzero and collaborators suggest that Kondo insulators such as SmB6 can be topological. Like SmB6, Cubic SmS is a non-magnetic semiconductor with an insulating behavior at ambient pressure and low temperatures driven by hybridization with the Sm f-electrons. At 6 kbar, SmS undergoes a phase transition into a valance fluctuating phase accompanied by a visible color change from black to gold. It then undergoes a second phase transition at about 20 kbar to an antiferromagnetic order at low temperatures. We will discuss whether electronic structure calculations indicate a topological state of SmS at P =0. We will also discuss whether or not the magnetic, thermal and transport properties of the black phase of SmS are consistent with the existence of a topological protected surface state.

  17. Dielectric relaxation, resonance and scaling behaviors in Sr3Co2Fe24O41 hexaferrite

    NASA Astrophysics Data System (ADS)

    Tang, Rujun; Jiang, Chen; Qian, Wenhu; Jian, Jie; Zhang, Xin; Wang, Haiyan; Yang, Hao

    2015-08-01

    The dielectric properties of Z-type hexaferrite Sr3Co2Fe24O41 (SCFO) have been investigated as a function of temperature from 153 to 503 K between 1 and 2 GHz. The dielectric responses of SCFO are found to be frequency dependent and thermally activated. The relaxation-type dielectric behavior is observed to be dominating in the low frequency region and resonance-type dielectric behavior is found to be dominating above 108 Hz. This frequency dependence of dielectric behavior is explained by the damped harmonic oscillator model with temperature dependent coefficients. The imaginary part of impedance (Z″) and modulus (M″) spectra show that there is a distribution of relaxation times. The scaling behaviors of Z″ and M″ spectra further suggest that the distribution of relaxation times is temperature independent at low frequencies. The dielectric loss spectra at different temperatures have not shown a scaling behavior above 108 Hz. A comparison between the Z″ and the M″ spectra indicates that the short-range charges motion dominates at low temperatures and the long-range charges motion dominates at high temperatures. The above results indicate that the dielectric dispersion mechanism in SCFO is temperature independent at low frequencies and temperature dependent at high frequencies due to the domination of resonance behavior.

  18. Dielectric relaxation, resonance and scaling behaviors in Sr3Co2Fe24O41 hexaferrite.

    PubMed

    Tang, Rujun; Jiang, Chen; Qian, Wenhu; Jian, Jie; Zhang, Xin; Wang, Haiyan; Yang, Hao

    2015-08-28

    The dielectric properties of Z-type hexaferrite Sr3Co2Fe24O41 (SCFO) have been investigated as a function of temperature from 153 to 503 K between 1 and 2 GHz. The dielectric responses of SCFO are found to be frequency dependent and thermally activated. The relaxation-type dielectric behavior is observed to be dominating in the low frequency region and resonance-type dielectric behavior is found to be dominating above 10(8) Hz. This frequency dependence of dielectric behavior is explained by the damped harmonic oscillator model with temperature dependent coefficients. The imaginary part of impedance (Z″) and modulus (M″) spectra show that there is a distribution of relaxation times. The scaling behaviors of Z″ and M″ spectra further suggest that the distribution of relaxation times is temperature independent at low frequencies. The dielectric loss spectra at different temperatures have not shown a scaling behavior above 10(8) Hz. A comparison between the Z″ and the M″ spectra indicates that the short-range charges motion dominates at low temperatures and the long-range charges motion dominates at high temperatures. The above results indicate that the dielectric dispersion mechanism in SCFO is temperature independent at low frequencies and temperature dependent at high frequencies due to the domination of resonance behavior.

  19. Dielectric relaxation, resonance and scaling behaviors in Sr3Co2Fe24O41 hexaferrite

    PubMed Central

    Tang, Rujun; Jiang, Chen; Qian, Wenhu; Jian, Jie; Zhang, Xin; Wang, Haiyan; Yang, Hao

    2015-01-01

    The dielectric properties of Z-type hexaferrite Sr3Co2Fe24O41 (SCFO) have been investigated as a function of temperature from 153 to 503 K between 1 and 2 GHz. The dielectric responses of SCFO are found to be frequency dependent and thermally activated. The relaxation-type dielectric behavior is observed to be dominating in the low frequency region and resonance-type dielectric behavior is found to be dominating above 108 Hz. This frequency dependence of dielectric behavior is explained by the damped harmonic oscillator model with temperature dependent coefficients. The imaginary part of impedance (Z″) and modulus (M″) spectra show that there is a distribution of relaxation times. The scaling behaviors of Z″ and M″ spectra further suggest that the distribution of relaxation times is temperature independent at low frequencies. The dielectric loss spectra at different temperatures have not shown a scaling behavior above 108 Hz. A comparison between the Z″ and the M″ spectra indicates that the short-range charges motion dominates at low temperatures and the long-range charges motion dominates at high temperatures. The above results indicate that the dielectric dispersion mechanism in SCFO is temperature independent at low frequencies and temperature dependent at high frequencies due to the domination of resonance behavior. PMID:26314913

  20. Mesoscopic features in the transport properties of a Kondo-correlated quantum dot in a magnetic field.

    PubMed

    Camjayi, Alberto; Arrachea, Liliana

    2014-01-22

    We study the transport behavior induced by a small bias voltage through a quantum dot connected to one-channel finite-size wires. We describe the quantum dot using the Hubbard-Anderson impurity model and we obtain solutions by means of a quantum Monte Carlo method. We investigate the effect of a magnetic field applied at the quantum dot in the Kondo regime. We identify mesoscopic oscillations in the conductance, which are introduced by the magnetic field. This behavior is analogous to that observed as a function of the temperature.

  1. Resonant impurities and their electronic behavior in single-layer graphene

    NASA Astrophysics Data System (ADS)

    Wang, Lin

    The electronic behavior of single-layer graphene (SLG) containing resonant impurities wasinvestigated, particularly by quantum capacitance measurements. Before introducing resonant impurities into SLG, the properties of pristine SLG devices top-gated using ultra-thin Y2O3 dielectric layers were systematically studied by structure characterization, DC transport measurements and AC quantum capacitance measurements. Y2O 3 is an ideal candidate of dielectric materials for SLG top-gated devices by introducing very few short-range impurities. This facilitates us to probe the quantum capacitance and the density of states (D = Cq/e 2) of pristine and disordered graphene due to its very large capacitance. A new type of resonant impurities of Ag adatoms deposited on SLG was successfully detected through quantum capacitance measurements. The midgap states induced by Ag-adatoms are visible at room temperature and more evident at cryogenic temperatures. Theintensity of Ag-adatom-induced resonances becomes stronger at higher impurity concentration and higher magnetic fields, which agrees fairly well with theoretical calculations based on the density functional theory (DFT) and tight-binding model (TB). We elucidated that the appearance of the robust resonant peak near the charge neutrality point (CNP) and the splitting of zero Landau level (LL) for Ag-adsorbed graphene are manifestations of the hybridization effect of electrons from graphene bands and the resonant impurity bands. With a very high density of Ag adatoms, SLG capacitors show unconventional negative quantum capacitance behavior. The Ag adatoms act as resonant impurities and form nearly dispersionless resonant impurity bands near the CNP. Resonant impurities quench the kinetic energy and drive the electrons to the Coulomb energy dominated regime with negative compressibility. In the absence of a magnetic field, negative quantum capacitance is observed near the CNP. In the quantum Hall regime, negative quantum

  2. Topological defects of Néel order and Kondo singlet formation for Kondo-Heisenberg model on a honeycomb lattice

    NASA Astrophysics Data System (ADS)

    Si, Qimiao; Goswami, Pallab

    2014-03-01

    Heavy fermion systems represent a prototypical setting to study magnetic quantum phase transitions. In this context, we study the spin one-half Kondo-Heisenberg model on a honeycomb lattice at half filling. The problem is approached from the Kondo destroyed, antiferromagnetically ordered insulating phase. We describe the local moments in terms of a coarse grained quantum non-linear sigma model, and show that the skyrmion defects of the antiferromagnetic order parameter host a number of competing order parameters. In addition to the spin Peierls, charge and current density wave order parameters, we identify for the first time Kondo singlets as the competing dual orders of the antiferromagnetism, which can be related to each other via generalized chiral transformations of the underlying fermions. We also show that the conduction electrons acquire a Berry phase through their coupling to the hedgehog configurations of the Néel order, which cancels the Berry phase of the local moments. Our results demonstrate the competition between the Kondo-singlet formation and spin-Peierls order when the antiferromagnetic order is suppressed, thereby shedding new light on the global phase diagram of heavy fermion systems at zero temperature. NSF.

  3. Kondo spin liquid in the Kondo necklace model: Classical disordered phase versus symmetry-protected topological state

    NASA Astrophysics Data System (ADS)

    Zhong, Yin; Wang, Yu-Feng; Lu, Han-Tao; Luo, Hong-Gang

    2014-08-01

    We have studied Kondo spin liquid phase of Kondo necklace models from the perspective of quantum O(N) non-linear sigma model (NLSM) field theory, particularly we focus on its possible topologically nontrivial phases. In the one-dimensional case, the Kondo spin liquid phase is a usual quantum disordered phase in contrast to the well-known topologically nontrivial Haldane phase due to destructive interference effect of topological θ term. In the two-dimensional case, the system can be mapped onto an O(4)-like NLSM with some O(3) anisotropy. Interestingly, if hedgehog-like point defects are included together with the restoration of the full O(4) symmetry, our model is identical to a kind of SU(2) symmetry-protected topological (SPT) state, which highlights a possible link between the extended Kondo necklace models and the desirable SPT states. Additionally, if the system has the expanded O(5) symmetry instead, the effective NLSM with the Wess-Zumino-Witten term is just a description of the surface modes of a three-dimensional SPT state. The deviations from fully symmetrical cases are discussed. We expect that the results might provide useful threads to identify certain microscopic bilayer antiferromagnet models (and related materials), which can support the SPT states.

  4. Unconventional bulk three-dimensional Fermi surface in Kondo insulating SmB6

    NASA Astrophysics Data System (ADS)

    Tan, Beng

    We report the observation of a paradoxical insulator with a bulk state which is electrically insulating and simultaneously yields quantum oscillations typical of good metals. We present high field measurements of conductivity and magnetic torque in high purity single crystals of the Kondo insulator SmB6 which reveal an activated behavior characteristics of an insulator with an energy gap at the Fermi energy in the former and quantum oscillation of frequencies characteristics of a large three-dimensional conduction electron Fermi surface similar to the metallic rare earth hexaborides such as PrB6 and LaB6 in the latter. The quantum oscillations observed in the magnetic torque measurements are characteristic of an unconventional Fermi liquid - the amplitude strongly increases at low temperatures in a stark contrast to the saturating Lifshitz-Kosevich behavior in conventional metallic states.

  5. Kondo effect of D\\xAFs and D\\xAFs* mesons in nuclear matter

    NASA Astrophysics Data System (ADS)

    Yasui, Shigehiro; Sudoh, Kazutaka

    2017-03-01

    We study the Kondo effect for D¯s and D¯s* mesons as impurity particles in nuclear matter. The spin-exchange interaction between the D¯s or D¯s* meson and the nucleon induces the enhancement of the effective coupling in the low-energy scattering in the infrared region, whose energy scale of singularity is given by the Kondo scale. We investigate the Kondo scale in the renormalization group equation at nucleon one-loop level. We furthermore study the ground state with the Kondo effect in the mean-field approach, and present that the Kondo scale is related to the mixing strength between the D¯s or D¯s* meson and the nucleon in nuclear matter. We show the spectral function of the impurity when the Kondo effect occurs.

  6. Theory of Kondo suppression of spin polarization in nonlocal spin valves

    NASA Astrophysics Data System (ADS)

    Kim, K.-W.; O'Brien, L.; Crowell, P. A.; Leighton, C.; Stiles, M. D.

    2017-03-01

    We theoretically analyze contributions from the Kondo effect to the spin polarization and spin diffusion length in all-metal nonlocal spin valves. Interdiffusion of ferromagnetic atoms into the normal metal layer creates a region in which Kondo physics plays a significant role, giving discrepancies between experiment and existing theory. We start from a simple model and construct a modified spin drift-diffusion equation which clearly demonstrates how the Kondo physics not only suppresses the electrical conductivity but even more strongly reduces the spin diffusion length. We also present an explicit expression for the suppression of spin polarization due to Kondo physics in an illustrative regime. We compare this theory to previous experimental data to extract an estimate of the Elliot-Yafet probability for Kondo spin flip scattering of 0.7 ±0.4 , in good agreement with the value of 2/3 derived in the original theory of Kondo.

  7. Many-terminal Majorana island: From topological to multichannel Kondo model

    NASA Astrophysics Data System (ADS)

    Herviou, Loïc; Le Hur, Karyn; Mora, Christophe

    2016-12-01

    We study Kondo screening obtained by coupling Majorana bound states, located on a topological superconducting island, to interacting electronic reservoirs. At the charge degeneracy points of the island, we formulate an exact mapping onto the spin-1 /2 multichannel Kondo effect. The coupling to Majorana fermions transforms the tunneling terms into effective fermionic bilinear contributions with a Luttinger parameter K in the leads that is effectively doubled. For strong interactions K =1 /2 , the intermediate fixed point of the standard multichannel Kondo model is exactly recovered. It evolves with K and connects to strong coupling in the noninteracting case K =1 , with maximum conductance between the leads and robustness against channel asymmetries similarly to the topological Kondo effect. For a number of leads above four, there exists a window of Luttinger parameters in which a quantum phase transition can occur between the strong coupling topological Kondo state and the partially conducting multichannel Kondo state.

  8. Resonant behavior of a harmonic oscillator with fluctuating mass driven by a Mittag-Leffler noise

    NASA Astrophysics Data System (ADS)

    Zhong, Suchuan; Yang, Jianqiang; Zhang, Lu; Ma, Hong; Luo, Maokang

    2017-02-01

    The resonant behavior of a generalized Langevin equation (GLE) in the presence of a Mittag-Leffler noise is studied analytically in this paper. Considering that a GLE with a Mittag-Leffler friction kernel is very useful for modeling anomalous diffusion processes with long-memory and long-range dependence, and the surrounding molecules do not only collide with the Brownian particle but also adhere to the Brownian particle for random time. Thus, we consider the Brownian particle with fluctuating mass, and the fluctuations of the mass are modelled as a dichotomous noise. Applying the stochastic averaging method, we obtain the exact expression of the output amplitude gain of the system. By studying the impact of the driving frequency and the noise parameters, we find the non-monotonic behaviors of the output amplitude gain. The results indicate that the bona fide SR, the wide sense SR and the conventional SR phenomena occur in the proposed harmonic oscillator with fluctuating mass driven by Mittag-Leffler noise. It is found that when we consider the output amplitude gain versus the driving frequency, the phenomena of stochastic multi-resonance (SMR) with two, three and four peaks are observed, and the quadruple-peaks SR phenomenon had never been observed in previous literature. Besides, when we investigate the dependence of output amplitude gain on the memory exponent, the inverse stochastic resonance (ISR) phenomenon takes place, in contrast to the well-known phenomenon of stochastic resonance. Furthermore, we compare the corresponding ordinary harmonic oscillator without memory to our generalized model, and found that the properties of long-memory and long-range dependence endows our generalized model with more abundant dynamic behaviors than the ordinary harmonic oscillator without memory.

  9. Model for overscreened Kondo effect in ultracold Fermi gas

    NASA Astrophysics Data System (ADS)

    Kuzmenko, I.; Kuzmenko, T.; Avishai, Y.; Kikoin, K.

    2015-04-01

    The feasibility of realizing the overscreened Kondo effect in ultracold Fermi gas of atoms with spin s ≥ 3/2 in the presence of a localized magnetic impurity atom is proved realistic. Specifying (as a mere example) a system of ultracold 22Na Fermi gas and a trapped 6Li impurity, the mechanism of exchange interaction between the Na and Li atoms is elucidated and the exchange constant is found to be positive (antiferromagnetic). The corresponding exchange Hamiltonian is derived, and the Kondo temperature is estimated at the order of 500 nK. Within a weak-coupling renormalization group scheme, it is shown that the coupling renormalizes to the non-Fermi-liquid fixed point. An observable displaying multichannel features even in the weak-coupling regime is the impurity magnetization that is negative for T ≫TK and becomes positive with decreasing temperature.

  10. Diagonal composite order in a two-channel Kondo lattice.

    PubMed

    Hoshino, Shintaro; Otsuki, Junya; Kuramoto, Yoshio

    2011-12-09

    A novel type of symmetry breaking is reported for the two-channel Kondo lattice where conduction electrons have spin and orbital (channel) degrees of freedom. Using the continuous-time quantum Monte Carlo and the dynamical mean-field theory, a spontaneous breaking of the orbital symmetry is observed. The tiny breakdown of orbital occupation number, however, vanishes if the conduction electrons have the particle-hole symmetry. The proper order parameter instead is identified as a composite quantity representing the orbital-selective Kondo effect. The single-particle spectrum of the selected orbital shows insulating property, while the other orbital behaves as a Fermi liquid. This composite order is the first example of odd-frequency order other than off-diagonal order (superconductivity), and is a candidate of hidden order in f-electron systems.

  11. Characterization of a correlated topological Kondo insulator in one dimension

    NASA Astrophysics Data System (ADS)

    Hagymási, I.; Legeza, Ö.

    2016-04-01

    We investigate the ground state of a p -wave Kondo-Heisenberg model introduced by Alexandrov and Coleman with an Ising-type anisotropy in the Kondo interaction and correlated conduction electrons. Our aim is to understand how they affect the stability of the Haldane state obtained in the SU(2)-symmetric case without the Hubbard interaction. By applying the density-matrix renormalization group algorithm and calculating the entanglement entropy we show that in the anisotropic case a phase transition occurs and a Néel state emerges above a critical value of the Coulomb interaction. These findings are also corroborated by the examination of the entanglement spectrum and the spin profile of the system which clarify the structure of each phase.

  12. The Spin Glass-Kondo Competition in Disordered Cerium Systems

    NASA Astrophysics Data System (ADS)

    Magalhaes, S. G.; Zimmer, F.; Coqblin, B.

    2013-10-01

    We discuss the competition between the Kondo effect, the spin glass state and a magnetic order observed in disordered Cerium systems. We present firstly the experimental situation of disordered alloys such as CeNi1 - xCux and then the different theoretical approaches based on the Kondo lattice model, with different descriptions of the intersite exchange interaction for the spin glass. After the gaussian approach of the Sherrington-Kirkpatrick model, we discuss the Mattis and the van Hemmen models. Then, we present simple cluster calculations in order to describe the percolative evolution of the clusters from the cluster spin glass to the inhomogeneous ferromagnetic order recently observed in CeNi1 - xCux disordered alloys and finally we discuss the effect of random and transverse magnetic field.

  13. Switchable Multiple Spin States in the Kondo description of Doped Molecular Magnets.

    PubMed

    Ray, Rajyavardhan; Kumar, Sanjeev

    2017-02-08

    We show that introducing electrons in magnetic clusters and molecular magnets lead to rich phase diagrams with a variety of low-spin and high-spin states allowing for multiple switchability. The analysis is carried out for a quantum spin-fermion model using the exact diagonalization, and the cluster mean-field approach. The model is relevant for a number of molecular magnets with triangular motifs consisting of transition metal ions such as Cr, Cu and V. Re-entrant spin-state behavior and chirality on-off transitions exist over a wide parameter regime. A subtle competition among geometrical frustration effects, electron itinerancy, and Kondo coupling at the molecular level is highlighted. Our results demonstrate that electron doping provides a viable mean to tame the magnetic properties of molecular magnets towards potential technological applications.

  14. Universal low-temperature crossover in two-channel Kondo models

    NASA Astrophysics Data System (ADS)

    Mitchell, Andrew K.; Sela, Eran

    2012-06-01

    An exact expression is derived for the electron Green function in two-channel Kondo models with one and two impurities, describing the crossover from non-Fermi liquid (NFL) behavior at intermediate temperatures to standard Fermi liquid (FL) physics at low temperatures. Symmetry-breaking perturbations generically present in experiment ensure the standard low-energy FL description, but the full crossover is wholly characteristic of the unstable NFL state. Distinctive conductance lineshapes in quantum dot devices should result. We exploit a connection between this crossover and one occurring in a classical boundary Ising model to calculate real-space electron densities at finite temperature. The single universal finite-temperature Green function is then extracted by inverting the integral transformation relating these Friedel oscillations to the t matrix. Excellent agreement is demonstrated between exact results and full numerical renormalization group calculations.

  15. Switchable Multiple Spin States in the Kondo description of Doped Molecular Magnets

    PubMed Central

    Ray, Rajyavardhan; Kumar, Sanjeev

    2017-01-01

    We show that introducing electrons in magnetic clusters and molecular magnets lead to rich phase diagrams with a variety of low-spin and high-spin states allowing for multiple switchability. The analysis is carried out for a quantum spin-fermion model using the exact diagonalization, and the cluster mean-field approach. The model is relevant for a number of molecular magnets with triangular motifs consisting of transition metal ions such as Cr, Cu and V. Re-entrant spin-state behavior and chirality on-off transitions exist over a wide parameter regime. A subtle competition among geometrical frustration effects, electron itinerancy, and Kondo coupling at the molecular level is highlighted. Our results demonstrate that electron doping provides a viable mean to tame the magnetic properties of molecular magnets towards potential technological applications. PMID:28176869

  16. Interfacial phase competition induced Kondo-like effect in manganite-insulator composites

    NASA Astrophysics Data System (ADS)

    Lin, Ling-Fang; Wu, Ling-Zhi; Dong, Shuai

    2016-12-01

    A Kondo-like effect, namely, the upturn of resistivity at low temperatures, is observed in perovskite manganite when nonmagnetic insulators are doped as secondary phase. In this paper, the low-temperature resistivity upturn effect has been argued to originate from interfacial magnetic phase reconstruction. Heisenberg spin lattices have been simulated using the Monte Carlo method to reveal phase competition around secondary phase boundary, namely, manganite-insulator boundary that behaves with a weak antiferromagnetic tendency. Moreover, the resistor network model based on double-exchange conductive mechanism reproduces the low-temperature resistivity upturn effect. Our work provides a reasonable physical mechanism to understand the novel transport behaviors in microstructures of correlated electron systems.

  17. Kondo effect in CoxCu1-x granular alloys prepared by chemical reduction method

    NASA Astrophysics Data System (ADS)

    Dhara, Susmita; Chowdhury, Rajeswari Roy; Bandyopadhyay, Bilwadal

    2015-06-01

    Nanostructured CoCu granular alloys CoxCu1-x (x ≤ 0.3) have been prepared by chemical reduction method using NaBH4 as a reducing agent. Electronic transport properties are studied in the temperature range 4-300 K. Resistance exhibits a metallic behavior below room temperature and draws a minimum near 20 K in all the samples except in Co0.3Cu0.7. This low temperature resistivity minimum diminishes with applied magnetic field. There is also a logarithmic temperature dependence of resistivity at temperatures below 20 K. This phenomenon indicates a Kondo-like scattering mechanism involving magnetic Co impurity spin clusters in Cu host.

  18. Switchable Multiple Spin States in the Kondo description of Doped Molecular Magnets

    NASA Astrophysics Data System (ADS)

    Ray, Rajyavardhan; Kumar, Sanjeev

    2017-02-01

    We show that introducing electrons in magnetic clusters and molecular magnets lead to rich phase diagrams with a variety of low-spin and high-spin states allowing for multiple switchability. The analysis is carried out for a quantum spin-fermion model using the exact diagonalization, and the cluster mean-field approach. The model is relevant for a number of molecular magnets with triangular motifs consisting of transition metal ions such as Cr, Cu and V. Re-entrant spin-state behavior and chirality on-off transitions exist over a wide parameter regime. A subtle competition among geometrical frustration effects, electron itinerancy, and Kondo coupling at the molecular level is highlighted. Our results demonstrate that electron doping provides a viable mean to tame the magnetic properties of molecular magnets towards potential technological applications.

  19. Universal out-of-equilibrium transport in Kondo-correlated quantum dots: renormalized dual fermions on the Keldysh contour.

    PubMed

    Muñoz, Enrique; Bolech, C J; Kirchner, Stefan

    2013-01-04

    The nonlinear conductance of semiconductor heterostructures and single molecule devices exhibiting Kondo physics has recently attracted attention. We address the observed sample dependence of the measured steady state transport coefficients by considering additional electronic contributions in the effective low-energy model underlying these experiments that are absent in particle-hole symmetric setups. A novel version of the superperturbation theory of Hafermann et al. in terms of dual fermions is developed, which correctly captures the low-temperature behavior. We compare our results with the measured transport coefficients.

  20. Antiferromagnetic Kondo lattice compound CePt3P

    PubMed Central

    Chen, Jian; Wang, Zhen; Zheng, Shiyi; Feng, Chunmu; Dai, Jianhui; Xu, Zhu’an

    2017-01-01

    A new ternary platinum phosphide CePt3P was synthesized and characterized by means of magnetic, thermodynamic and transport measurements. The compound crystallizes in an antiperovskite tetragonal structure similar to that in the canonical family of platinum-based superconductors APt3P (A = Sr, Ca, La) and closely related to the noncentrosymmetric heavy fermion superconductor CePt3Si. In contrast to all the superconducting counterparts, however, no superconductivity is observed in CePt3P down to 0.5 K. Instead, CePt3P displays a coexistence of antiferromagnetic ordering, Kondo effect and crystalline electric field effect. A field-induced spin-flop transition is observed below the magnetic ordering temperature TN1 of 3.0 K while the Kondo temperature is of similar magnitude as TN1. The obtained Sommerfeld coefficient of electronic specific heat is γCe = 86 mJ/mol·K2 indicating that CePt3P is a moderately correlated antiferromagnetic Kondo lattice compound. PMID:28157184

  1. Kondo physics from quasiparticle poisoning in Majorana devices

    DOE PAGES

    Plugge, S.; Tsvelik, A. M.; Zazunov, A.; ...

    2016-03-24

    Here, we present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M = 2 attached leads, such “dangerous” quasiparticle poisoning processes cause a spin S = 1/2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effectmore » of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, for M > 3, the topological Kondo fixed point re-emerges, though now it involves only M–1 leads. As a consequence, for M = 3, the low-energy fixed point becomes trivial corresponding to decoupled leads.« less

  2. Kondo physics from quasiparticle poisoning in Majorana devices

    SciTech Connect

    Plugge, S.; Tsvelik, A. M.; Zazunov, A.; Eriksson, E.; Egger, R.

    2016-03-24

    Here, we present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M = 2 attached leads, such “dangerous” quasiparticle poisoning processes cause a spin S = 1/2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effect of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, for M > 3, the topological Kondo fixed point re-emerges, though now it involves only M–1 leads. As a consequence, for M = 3, the low-energy fixed point becomes trivial corresponding to decoupled leads.

  3. Kondo physics from quasiparticle poisoning in Majorana devices

    NASA Astrophysics Data System (ADS)

    Plugge, S.; Zazunov, A.; Eriksson, E.; Tsvelik, A. M.; Egger, R.

    2016-03-01

    We present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M =2 attached leads, such "dangerous" quasiparticle poisoning processes cause a spin S =1 /2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effect of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, for M >3 , the topological Kondo fixed point re-emerges, though now it involves only M -1 leads. As a consequence, for M =3 , the low-energy fixed point becomes trivial corresponding to decoupled leads.

  4. Kondo correlations formation and the local magnetic moment dynamics in the Anderson model

    NASA Astrophysics Data System (ADS)

    Maslova, N. S.; Arseyev, P. I.; Mantsevich, V. N.

    2017-02-01

    We investigated the typical time scales of the Kondo correlations formation for the single-state Anderson model, when coupling to the reservoir is switched on at the initial time moment. The influence of the Kondo effect appearance on the system non-stationary characteristics was analyzed and discussed.

  5. Quantum phase transitions and anomalous Hall effect in a pyrochlore Kondo lattice

    NASA Astrophysics Data System (ADS)

    Grefe, Sarah; Ding, Wenxin; Si, Qimiao

    The metallic variant of the pyrochlore iridates Pr2Ir2O7 has shown characteristics of a possible chiral spin liquid state [PRL 96 087204 (2006), PRL 98, 057203 (2007), Nature 463, 210 (2010)] and quantum criticality [Nat. Mater. 13, 356 (2014)]. An important question surrounding the significant anomalous Hall response observed in Pr2Ir2O7 is the nature of the f-electron local moments, including their Kondo coupling with the conduction d-electrons. The heavy effective mass and related thermodynamic characteristics indicate the involvement of the Kondo effect in this system's electronic properties. In this work, we study the effects of Kondo coupling on candidate time-reversal-symmetry-breaking spin liquid states on the pyrochlore lattice. Representing the f-moments as slave fermions Kondo-coupled to conduction electrons, we study the competition between Kondo-singlet formation and chiral spin correlations and determine the zero-temperature phase diagram. We derive an effective chiral interaction between the local moments and the conduction electrons and calculate the anomalous Hall response across the quantum phase transition from the Kondo destroyed phase to the Kondo screened phase. We discuss our results' implications for Pr2Ir2O7 and related frustrated Kondo-lattice systems.

  6. Modeling the nuclear magnetic resonance behavior of lung: from electrical engineering to critical care medicine.

    PubMed

    Cutillo, A G; Ailion, D C

    1999-01-01

    The present article reviews the basic principles of a new approach to the characterization of pulmonary disease. This approach is based on the unique nuclear magnetic resonance (NMR) properties of the lung and combines experimental measurements (using specially developed NMR techniques) with theoretical simulations. The NMR signal from inflated lungs decays very rapidly compared with the signal from completely collapsed (airless) lungs. This phenomenon is due to the presence of internal magnetic field inhomogeneity produced by the alveolar air-tissue interface (because air and water have different magnetic susceptibilities). The air-tissue interface effects can be detected and quantified by magnetic resonance imaging (MRI) techniques using temporally symmetric and asymmetric spin-echo sequences. Theoretical models developed to explain the internal (tissue-induced) magnetic field inhomogeneity in aerated lungs predict the NMR lung behavior as a function of various technical and physiological factors (e.g., the level of lung inflation) and simulate the effects of various lung disorders (in particular, pulmonary edema) on this behavior. Good agreement has been observed between the predictions obtained from the mathematical models and the results of experimental NMR measurements in normal and diseased lungs. Our theoretical and experimental data have important pathophysiological and clinical implications, especially with respect to the characterization of acute lung disease (e.g., pulmonary edema) and the management of critically ill patients.

  7. Fermionology in the Kondo-Heisenberg model: the case of CeCoIn5

    NASA Astrophysics Data System (ADS)

    Zhong, Yin; Zhang, Lan; Lu, Han-Tao; Luo, Hong-Gang

    2015-09-01

    The Fermi surface of heavy electron systems plays a fundamental role in understanding their variety of puzzling phenomena, for example, quantum criticality, strange metal behavior, unconventional superconductivity and even enigmatic phases with yet unknown order parameters. The spectroscopy measurement of the typical heavy fermion superconductor CeCoIn5 has demonstrated multi-Fermi surface structure, which has not been studied in detail theoretically in a model system like the Kondo-Heisenberg model. In this work, we take a step toward such a theoretical model by revisiting the Kondo-Heisenberg model. It is found that the usual self-consistent calculation cannot reproduce the fermionology of the experimental observation of the system due to the sign binding between the hopping of the conduction electrons and the mean-field valence-bond order. To overcome such inconsistency, the mean-field valence-bond order is considered as a free/fitting parameter to correlate them with real-life experiments as performed in recent experiments [M.P. Allan, F. Massee, D.K. Morr, J. Van Dyke, A.W. Rost, A.P. Mackenzie, C. Petrovic, J.C. Davis, Nat. Phys. 9, 468 (2013); J. Van Dyke, F. Massee, M.P. Allan, J.C. Davis, C. Petrovic, D.K. Morr, Proc. Natl. Acad. Sci. 111, 11663 (2014)], which also explicitly reflects the intrinsic dispersion of local electrons observed in experimental measurements. Given the fermionology, the calculated effective mass enhancement, entropy, superfluid density and Knight shift are all in qualitative agreement with the experimental results of CeCoIn5, which confirms our assumption. Our result supports a d_{x^2 - y^2 }-wave pairing structure in the heavy fermion material CeCoIn5.

  8. Theory of the orbital Kondo effect with assisted hopping in strongly correlated electron systems: Parquet equations, superconductivity, and mass enhancement

    NASA Astrophysics Data System (ADS)

    Penc, K.; Zawadowski, A.

    1994-10-01

    The orbital Kondo effect is treated in a model where, additional to the conduction band, there are localized orbitals close to the Fermi energy. If the hopping between the conduction band and the localized heavy orbitals depends on the occupation of the atomic orbitals in the conduction band, then orbital Kondo correlation occurs. The noncommutative nature of the coupling required for the Kondo effect is formally due to the form factors associated with the assisted hopping, which in the momentum representation depends on the momenta of the conduction electrons involved. The leading logarithmic vertex corrections are due to the local Coulomb interaction between the electrons on the heavy orbital and in the conduction band. The renormalized vertex functions are obtained as a solution of a closed set of differential equations and they show power behavior. The amplitude of large renormalization is determined by an infrared cutoff due to finite energy and dispersion of the heavy particles. The enhanced assisted hopping rate results in mass enhancement and attractive interaction in the conduction band. The superconductivity transition temperature calculated is largest for the intermediate mass enhancement, m*/m~=2-3. For larger mass enhancement the small one-particle weight (Z) in the Green's function reduces the transition temperature, which may be characteristic for other models as well. The theory is developed for different one-dimensional and square-lattice models, but the applicability is not limited to them. In the one-dimensional case charge- and spin-density susceptibilities are also discussed. Good candidates for the heavy orbital are f bands in the heavy fermionic systems and nonbonding oxygen orbitals in high-temperature superconductors and different flatbands in the quasi-one-dimensional organic conductors.

  9. Resonances and resonance widths

    SciTech Connect

    Collins, T.

    1986-05-01

    Two-dimensional betatron resonances are much more important than their simple one-dimensional counterparts and exhibit a strong dependence on the betatron phase advance per cell. A practical definition of ''width'' is expanded upon in order to display these relations in tables. A primarily pedagogical introduction is given to explain the tables, and also to encourage a wider capability for deriving resonance behavior and wider use of ''designer'' resonances.

  10. Chaotic Behavior Near First-order Mean Motion Resonances in the Elliptical, Planar Three Body Problem

    NASA Astrophysics Data System (ADS)

    El Moutamid, Maryame; Sicardy, B.; Renner, S.

    2013-05-01

    Abstract (2,250 Maximum Characters): We investigate the behavior of two bodies μ and μ' orbiting a massive central body in a common plane, near a first order mean motion resonance m+1:m, where m is an integer. We obtain a system with two critical resonant angles φ = (m+1)λ' -mλ - ω and φ' = (m+1)λ' -mλ - ω', where λ and ω are the mean longitude and the longitude of periapsis of μ, respectively, and the primed quantities apply to μ'. The aims of the presentation is (1) to discuss the integrability of this two-degree of freedom system. When there are no secular precession terms, the integrability of the system stems from the existence of a second integral of motion, besides the Hamiltonian. We show that this second integral is a modified version of the Jacobi constant, where the orbital eccentricity of μ (or μ') is replaced by the relative eccentricity between the two orbits. When the central potential is not anymore Keplerian (due for instance to the oblateness of the central body), then the differential orbital precession of μ and μ' destroys that modified Jacobi constant. The second goal is (2) to rescale the restricted problem (μ = 0) so that it depends upon two parameters only: the distance between the two resonances and the mass of μ'. While the problem is integrable when the distance is zero, we show numerically that a chaotic motion appears when the distance is small and different from zero. For large distances, the system tends again toward an integrable system solved using adiabatic invariance arguments.

  11. Modeling electromagnetic fields detectability in a HH-like neuronal system: stochastic resonance and window behavior.

    PubMed

    Giannì, Matteo; Liberti, Micaela; Apollonio, Francesca; D'Inzeo, Guglielmo

    2006-02-01

    Noise has already been shown to play a constructive role in neuronal processing and reliability, according to stochastic resonance (SR). Here another issue is addressed, concerning noise role in the detectability of an exogenous signal, here representing an electromagnetic (EM) field. A Hodgkin-Huxley like neuronal model describing a myelinated nerve fiber is proposed and validated, excited with a suprathreshold stimulation. EM field is introduced as an additive voltage input and its detectability in neuronal response is evaluated in terms of the output signal-to-noise ratio. Noise intensities maximizing spiking activity coherence with the exogenous EM signal are clearly shown, indicating a stochastic resonant behavior, strictly connected to the model frequency sensitivity. In this study SR exhibits a window of occurrence in the values of field frequency and intensity, which is a kind of effect long reported in bioelectromagnetic experimental studies. The spatial distribution of the modeled structure also allows to investigate possible effects on action potentials saltatory propagation, which results to be reliable and robust over the presence of an exogenous EM field and biological noise. The proposed approach can be seen as assessing biophysical bases of medical applications funded on electric and magnetic stimulation where the role of noise as a cooperative factor has recently gained growing attention.

  12. A nonferrous instrumental joystick device for recording behavioral responses during magnetic resonance imaging and spectroscopy.

    PubMed

    Lukas, S E; Dobrosielski, M; Chiu, T M; Woods, B T; Teoh, S K; Mendelson, J H

    1993-12-01

    A nonferrous joystick device was developed to permit subjects to continuously report ethanol-induced alterations in subjective mood states while undergoing a magnetic resonance imaging (MRI) and magnetic resonance spectroscopy (MRS) procedure. The device utilizes air pressure (supplied by a small compressor) that is directed to a series of tubes that terminate in a hand-held unit. The hand-held unit easily fits inside the magnet and resembles a standard computer game joystick except that the ends of the air hoses replace the buttons. The control unit contains three pressure transducers, which are triggered when the tubes are occluded by the subject, activating different pens on an event marker located 6 m from the whole body imager. The unit is safe to use inside a 1.5-Tesla magnetic field and does not disrupt the MRI and MRS recording procedures. Subjective reports of ethanol-induced euphoria and intoxication paralleled the MRS detection of ethanol in the brain. This device could prove to be useful in numerous behavioral studies involving whole-body MRI and MRS.

  13. Application of the S=1 underscreened Anderson lattice model to Kondo uranium and neptunium compounds

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simões, Acirete S.; Iglesias, J. R.; Lacroix, C.; Perkins, N. B.; Coqblin, B.

    2011-01-01

    Magnetic properties of uranium and neptunium compounds showing the coexistence of the Kondo screening effect and ferromagnetic order are investigated within the Anderson lattice Hamiltonian with a two-fold degenerate f level in each site, corresponding to 5f2 electronic configuration with S=1 spins. A derivation of the Schrieffer-Wolff transformation is presented and the resulting Hamiltonian has an effective f-band term, in addition to the regular exchange Kondo interaction between the S=1 f spins and the s=1/2 spins of the conduction electrons. The resulting effective Kondo lattice model can describe both the Kondo regime and a weak delocalization of the 5f electrons. Within this model we compute the Kondo and Curie temperatures as a function of model parameters, namely the Kondo exchange interaction constant JK, the magnetic intersite exchange interaction JH, and the effective f bandwidth. We deduce, therefore, a phase diagram of the model which yields the coexistence of the Kondo effect and ferromagnetic ordering and also accounts for the pressure dependence of the Curie temperature of uranium compounds such as UTe.

  14. Unveiling the internal entanglement structure of the Kondo singlet

    NASA Astrophysics Data System (ADS)

    Yang, Chun; Feiguin, Adrian E.

    2017-03-01

    We disentangle all the individual degrees of freedom in the quantum impurity problem to deconstruct the Kondo singlet, both in real and energy space, by studying the contribution of each individual free electron eigenstate. This is a problem of two spins coupled to a bath, where the bath is formed by the remaining conduction electrons. Being a mixed state, we resort to the "concurrence" to quantify entanglement. We identify "projected natural orbitals" that allow us to individualize a single-particle electronic wave function that is responsible of more than 90 % of the impurity screening. In the weak coupling regime, the impurity is entangled to an electron at the Fermi level, while in the strong coupling regime, the impurity counterintuitively entangles mostly with the high energy electrons and disentangles completely from the low-energy states carving a "hole" around the Fermi level. This enables one to use concurrence as a pseudo order parameter to compute the characteristic "size" of the Kondo cloud, beyond which electrons are weakly correlated to the impurity and are dominated by the physics of the boundary.

  15. Single- or multi-flavor Kondo effect in graphene

    NASA Astrophysics Data System (ADS)

    Zhu, Zhen-Gang; Ding, Kai-He; Berakdar, Jamal

    2010-06-01

    Based on the tight-binding formalism, we investigate the Anderson and the Kondo model for an adatom magnetic impurity above graphene. Different impurity positions are analyzed. Employing a partial-wave representation we study the nature of the coupling between the impurity and the conducting electrons. The components from the two Dirac points are mixed while interacting with the impurity. Two configurations are considered explicitly: the adatom is above one atom (ADA), the other case is the adatom above the center the honeycomb (ADC). For ADA the impurity is coupled with one flavor for both A and B sublattice and both Dirac points. For ADC the impurity couples with multi-flavor states for a spinor state of the impurity. We show, explicitly for a 3d magnetic atom, dz2, (dxz,dyz), and (dx2- y2,dxy) couple respectively with the Γ1, Γ5(E1), and Γ6(E2) representations (reps) of C6v group in ADC case. The bases for these reps of graphene are also derived explicitly. For ADA we calculate the Kondo temperature.

  16. Entanglement structure of the two-channel Kondo model

    NASA Astrophysics Data System (ADS)

    Alkurtass, Bedoor; Bayat, Abolfazl; Affleck, Ian; Bose, Sougato; Johannesson, Henrik; Sodano, Pasquale; Sørensen, Erik S.; Le Hur, Karyn

    2016-02-01

    Two electronic channels competing to screen a single impurity spin, as in the two-channel Kondo model, are expected to generate a ground state with a nontrivial entanglement structure. We exploit a spin-chain representation of the two-channel Kondo model to probe the ground-state block entropy, negativity, tangle, and Schmidt gap, using a density matrix renormalization group approach. In the presence of symmetric coupling to the two channels, we confirm field-theory predictions for the boundary entropy difference ln(gUV/gIR) =ln(2 ) /2 between the ultraviolet and infrared limits and the leading ln(x )/x impurity correction to the block entropy. The impurity entanglement Simp is shown to scale with the characteristic length ξ2 CK. We show that both the Schmidt gap and the entanglement of the impurity with one of the channels—as measured by the negativity—faithfully serve as order parameters for the impurity quantum phase transition appearing as a function of channel asymmetry, allowing for explicit determination of critical exponents, ν ≈2 and β ≈0.2 . Remarkably, we find the emergence of tripartite entanglement only in the vicinity of the critical channel-symmetric point.

  17. Interaction effect in the Kondo energy of the periodic Anderson-Hubbard model

    NASA Astrophysics Data System (ADS)

    Itai, K.; Fazekas, P.

    1996-07-01

    We extend the periodic Anderson model by switching on a Hubbard U for the conduction band. The nearly integral valent limit of the Anderson-Hubbard model is studied with the Gutzwiller variational method. The lattice Kondo energy shows U dependence both in the prefactor and the exponent. Switching on U reduces the Kondo scale, which can be understood to result from the blocking of hybridization. At half filling, we find a Brinkman-Rice-type transition from a Kondo insulator to a Mott insulator. Our findings should be relevant for a number of correlated two-band models of recent interest.

  18. Magnetic Flux Effect on a Kondo-Induced Electric Polarization in a Triangular Triple Quantum Dot

    NASA Astrophysics Data System (ADS)

    Koga, Mikito; Matsumoto, Masashige; Kusunose, Hiroaki

    2014-08-01

    A magnetic flux effect is studied theoretically on an electric polarization induced by the Kondo effect in a triangular triple-quantum-dot system, where one of the three dots is connected to a metallic lead. This electric polarization exhibits an Aharonov-Bohm oscillation as a function of the magnetic flux penetrating through the triangular loop. The numerical renormalization group analysis reveals how the oscillation pattern depends on the Kondo coupling of a local spin with lead electrons, which is sensitive to the point contact with the lead. It provides an experimental implication that the Kondo effect is the origin of the emergent electric polarization.

  19. Tunable pseudogap Kondo effect and quantum phase transitions in Aharonov-Bohm interferometers.

    PubMed

    Dias da Silva, Luis G G V; Sandler, Nancy; Simon, Pascal; Ingersent, Kevin; Ulloa, Sergio E

    2009-04-24

    We study two quantum dots embedded in the arms of an Aharonov-Bohm ring threaded by a magnetic flux. This system can be described by an effective one-impurity Anderson model with an energy- and flux-dependent density of states. For specific values of the flux, this density of states vanishes at the Fermi energy, yielding a controlled realization of the pseudogap Kondo effect. The conductance and transmission phase shifts reflect a nontrivial interplay between wave interference and interactions, providing clear signatures of quantum phase transitions between Kondo and non-Kondo ground states.

  20. Tunable Pseudogap Kondo Effect and Quantum Phase Transitions in Aharonov-Bohm Interferometers

    SciTech Connect

    Dias Da Silva, Luis G; Sandler, Nancy; Simon, Pascal; Ingersent, Kevin; Ulloa, Sergio E

    2009-01-01

    We study two quantum dots embedded in the arms of an Aharonov-Bohm ring threaded by a magnetic flux. This system can be described by an effective one-impurity Anderson model with an energy- and flux- dependent density of states. For specific values of the flux, this density of states vanishes at the Fermi energy, yielding a controlled realization of the pseudogap Kondo effect. The conductance and trans- mission phase shifts reflect a nontrivial interplay between wave interference and interactions, providing clear signatures of quantum phase transitions between Kondo and non-Kondo ground states.

  1. Magnetotransport study of Kondo compound Ce(Ni0.7Cu0.3)2Al3

    NASA Astrophysics Data System (ADS)

    Yadam, Sankararao; Singh, Durgesh; Venkateshwarlu, D.; Gangrade, Mohan Kumar; Samatham, S. Shanmukharao; Ganesan, V.

    2015-06-01

    CeNi2Al3 system has evolved in to a known thermoelectric material with a usable figure of merit at low temperatures. Kondo effect plays a crucial role in the enhancement of TEP in this system especially when the Ni site is substituted with non-magnetic elements like Cu. Effect of high magnetic fields on various properties of this system is yet to be explored. Ce(Ni0.7Cu0.3)2Al3 is a representative sample that has a significant enhancement of TEP whose reasons are being explored recently. Here we report the magnetoresistivity measurements on this sample down to 2K and fields upto 14T. The famous negative ln(T) rise with a minimum at 14.5 K is getting suppressed by the magnetic fields. Magnetic correlations are observed with increasing magnetic field strength in the form of a hump like behavior due to competition between Kondo and RKKY interactions. This hump is shifted to higher temperatures with increase in the field strength which indicates probable onset of ferromagnetic correlations that is being corroborated by the observed negative magnetoresistance at low temperatures.

  2. The resonance overlap criterion and the onset of stochastic behavior in the restricted three-body problem

    NASA Technical Reports Server (NTRS)

    Wisdom, J.

    1980-01-01

    The resonance overlap criterion for the onset of stochastic behavior is applied to the planar circular-restricted three-body problem with small mass ratio (mu). Its predictions for mu = 0.001, 0.0001, and 0.00001 are compared to the transitions observed in the numerically determined Kolmogorov-Sinai entropy and found to be in remarkably good agreement. In addition, an approximate scaling law for the onset of stochastic behavior is derived.

  3. Effects of Nonsphericity on the Behavior of Lorenz-Mie Resonances in Scattering Characteristics of Liquid-Cloud Droplets

    NASA Technical Reports Server (NTRS)

    Dlugach, Janna M.; Mishchenko, Michael I.

    2014-01-01

    By using the results of highly accurate T-matrix computations for randomly oriented oblate and prolate spheroids and Chebyshev particles with varying degrees of asphericity, we analyze the effects of a deviation of water-droplet shapes from that of a perfect sphere on the behavior of Lorenz-Mie morphology-dependent resonances of various widths. We demonstrate that the positions and profiles of the resonances can change significantly with increasing asphericity. The absolute degree of asphericity required to suppress a Lorenz-Mie resonance is approximately proportional to the resonance width. Our results imply that numerical averaging of scattering characteristics of real cloud droplets over sizes may rely on a significantly coarser size-parameter resolution than that required for ideal, perfectly spherical particles.

  4. Topological defects of Néel order and Kondo singlet formation for the Kondo-Heisenberg model on a honeycomb lattice

    NASA Astrophysics Data System (ADS)

    Goswami, Pallab; Si, Qimiao

    2014-01-01

    Heavy-fermion systems represent a prototypical setting to study magnetic quantum phase transitions. A particular focus has been on the physics of Kondo destruction, which captures quantum criticality beyond the Landau framework of order-parameter fluctuations. In this context, we study the spin one-half Kondo-Heisenberg model on a honeycomb lattice at half filling. The problem is approached from the Kondo-destroyed, antiferromagnetically ordered insulating phase. We describe the local moments in terms of a coarse grained quantum nonlinear sigma model, and show that the skyrmion defects of the antiferromagnetic order parameter host a number of competing order parameters. In addition to the spin Peierls, charge and current density wave order parameters, we identify for the first time Kondo singlets as the competing orders of the antiferromagnetism. We show that the antiferromagnetism and various competing singlet orders can be related to each other via generalized chiral transformations of the underlying fermions. We also show that the conduction electrons acquire a Berry phase through their coupling to the hedgehog configurations of the Néel order, which cancels the Berry phase of the local moments. Our results demonstrate the competition between the Kondo singlet formation and spin-Peierls order when the antiferromagnetic order is suppressed, thereby shedding new light on the global phase diagram of heavy-fermion systems at zero temperature.

  5. Theoretical analysis of 1D resonant tunneling behavior in ion-enhanced cold field and thermo-field emission

    NASA Astrophysics Data System (ADS)

    Tan, Xi; Rumbach, Paul; Griggs, Nathaniel; Jensen, Kevin L.; Go, David B.

    2016-12-01

    In cold field and thermo-field emission, positive ions or adsorbates very close to the cathode surface can enhance emission current by both resonant and non-resonant processes. In this paper, resonant tunneling behavior is investigated by solving the one-dimensional Schrödinger equation in the presence of an ion, and the enhancement due to resonant processes is evaluated. Results shows that as the applied electric field increases, the resonant states move from higher to lower energies as the ion energy levels are shifted down. Conversely, as the ion position moves closer to the cathode, the resonant states shift up in energy. Further, through a simplified perturbation analysis, the general scaling of these trends can be predicted. These shifts of resonant states directly impact the emission current density, and they are especially relevant when the applied field is on the order of a few volts per nanometer (˜0.5-3 V/nm) and the ion is a few nanometers (˜0.5-3 nm) away from the cathode. Further, when the energy level for resonant emission coincides with the Fermi level of a metallic cathode, the current density is particularly enhanced. The results of this study suggest that it may be possible to control (augment/inhibit) the resonant emission current by manipulating the supply function of a cathode relative to the operating conditions of the emitter in either ion-enhanced or adsorbate-enhanced field emission, which can be applied to various plasma and electron emission technologies.

  6. A theoretical study of the cluster glass-Kondo-magnetic disordered alloys

    NASA Astrophysics Data System (ADS)

    Zimmer, F. M.; Magalhães, S. G.; Coqblin, B.

    2009-10-01

    The physics of disordered alloys, such as typically the well known case of CeNi1-xCux alloys, showing an interplay among the Kondo effect, the spin glass state and a magnetic order, has been studied firstly within an average description like in the Sherrington-Kirkpatrick model. Recently, a theoretical model [S.G. Magalhaes, F.M. Zimmer, P.R. Krebs, B. Coqblin, Phys. Rev. B 74 (2006) 014427] involving a more local description of the intersite interaction has been proposed to describe the phase diagram of CeNi1-xCux. This alloy is an example of the complex interplay between Kondo effect and frustration in which there is in particular the onset of a cluster-glass state. Although the model given in Magalhaes et al. [Phys. Rev. B 74 (2006) 014427] has reproduced the different phases relatively well, it is not able to describe the cluster-glass state. We study here the competition between the Kondo effect and a cluster glass phase within a Kondo-lattice model with an inter-cluster random Gaussian interaction. The inter-cluster term is treated within the cluster mean-field theory for spin glasses [C.M. Sokoulis, Phys. Rev. B 18 (1978) 3757], while, inside the cluster, an exact diagonalisation is performed including inter-site ferromagnetic and intra-site Kondo interactions. The cluster glass order parameters and the Kondo correlation function are obtained for different values of the cluster size, the intra-cluster ferromagnetic coupling and the Kondo intra-site coupling. We obtain that the increase of the Kondo coupling tends clearly to destroy the cluster glass phase.

  7. How Kondo-holes create intense nanoscale heavy-fermion hybridization disorder

    PubMed Central

    Hamidian, Mohammad H.; Schmidt, Andrew R.; Firmo, Inês A.; Allan, Milan P.; Bradley, Phelim; Garrett, Jim D.; Williams, Travis J.; Luke, Graeme M.; Dubi, Yonatan; Balatsky, Alexander V.; Davis, J. C.

    2011-01-01

    Replacing a magnetic atom by a spinless atom in a heavy-fermion compound generates a quantum state often referred to as a “Kondo-hole”. No experimental imaging has been achieved of the atomic-scale electronic structure of a Kondo-hole, or of their destructive impact [Lawrence JM, et al. (1996) Phys Rev B 53:12559–12562] [Bauer ED, et al. (2011) Proc Natl Acad Sci. 108:6857–6861] on the hybridization process between conduction and localized electrons which generates the heavy-fermion state. Here we report visualization of the electronic structure at Kondo-holes created by substituting spinless thorium atoms for magnetic uranium atoms in the heavy-fermion system URu2Si2. At each thorium atom, an electronic bound state is observed. Moreover, surrounding each thorium atom we find the unusual modulations of hybridization strength recently predicted to occur at Kondo-holes [Figgins J, Morr DK (2011) Phys Rev Lett 107:066401]. Then, by introducing the “hybridization gapmap” technique to heavy-fermion studies, we discover intense nanoscale heterogeneity of hybridization due to a combination of the randomness of Kondo-hole sites and the long-range nature of the hybridization oscillations. These observations provide direct insight into both the microscopic processes of heavy-fermion forming hybridization and the macroscopic effects of Kondo-hole doping. PMID:22006302

  8. How Kondo-holes create intense nanoscale heavy-fermion hybridization disorder.

    PubMed

    Hamidian, Mohammad H; Schmidt, Andrew R; Firmo, Inês A; Allan, Milan P; Bradley, Phelim; Garrett, Jim D; Williams, Travis J; Luke, Graeme M; Dubi, Yonatan; Balatsky, Alexander V; Davis, J C

    2011-11-08

    Replacing a magnetic atom by a spinless atom in a heavy-fermion compound generates a quantum state often referred to as a "Kondo-hole". No experimental imaging has been achieved of the atomic-scale electronic structure of a Kondo-hole, or of their destructive impact [Lawrence JM, et al. (1996) Phys Rev B 53:12559-12562] [Bauer ED, et al. (2011) Proc Natl Acad Sci. 108:6857-6861] on the hybridization process between conduction and localized electrons which generates the heavy-fermion state. Here we report visualization of the electronic structure at Kondo-holes created by substituting spinless thorium atoms for magnetic uranium atoms in the heavy-fermion system URu(2)Si(2). At each thorium atom, an electronic bound state is observed. Moreover, surrounding each thorium atom we find the unusual modulations of hybridization strength recently predicted to occur at Kondo-holes [Figgins J, Morr DK (2011) Phys Rev Lett 107:066401]. Then, by introducing the "hybridization gapmap" technique to heavy-fermion studies, we discover intense nanoscale heterogeneity of hybridization due to a combination of the randomness of Kondo-hole sites and the long-range nature of the hybridization oscillations. These observations provide direct insight into both the microscopic processes of heavy-fermion forming hybridization and the macroscopic effects of Kondo-hole doping.

  9. Fractionalized Fermi liquid in a Kondo-Heisenberg model

    DOE PAGES

    Tsvelik, A. M.

    2016-10-10

    The Kondo-Heisenberg model is used as a controllable tool to demonstrate the existence of a peculiar metallic state with unbroken translational symmetry where the Fermi surface volume is not controlled by the total electron density. Here, I use a nonperturbative approach where the strongest interactions are taken into account by means of exact solution, and corrections are controllable. The resulting metallic state represents a fractionalized Fermi liquid where well defined quasiparticles coexist with gapped fractionalized collective excitations, in agreement with the general requirements formulated by T. Senthil et al. [Phys. Rev. Lett. 90, 216403 (2003)]. Furthermore, the system undergoes amore » phase transition to an ordered phase (charge density wave or superconducting), at the transition temperature which is parametrically small in comparison to the quasiparticle Fermi energy.« less

  10. Kondo Breakdown and Quantum Oscillations in SmB_{6}.

    PubMed

    Erten, Onur; Ghaemi, Pouyan; Coleman, Piers

    2016-01-29

    Recent quantum oscillation experiments on SmB_{6} pose a paradox, for while the angular dependence of the oscillation frequencies suggest a 3D bulk Fermi surface, SmB_{6} remains robustly insulating to very high magnetic fields. Moreover, a sudden low temperature upturn in the amplitude of the oscillations raises the possibility of quantum criticality. Here we discuss recently proposed mechanisms for this effect, contrasting bulk and surface scenarios. We argue that topological surface states permit us to reconcile the various data with bulk transport and spectroscopy measurements, interpreting the low temperature upturn in the quantum oscillation amplitudes as a result of surface Kondo breakdown and the high frequency oscillations as large topologically protected orbits around the X point. We discuss various predictions that can be used to test this theory.

  11. Kondo Breakdown and Quantum Oscillations in SmB6

    NASA Astrophysics Data System (ADS)

    Erten, Onur; Ghaemi, Pouyan; Coleman, Piers

    2016-01-01

    Recent quantum oscillation experiments on SmB6 pose a paradox, for while the angular dependence of the oscillation frequencies suggest a 3D bulk Fermi surface, SmB6 remains robustly insulating to very high magnetic fields. Moreover, a sudden low temperature upturn in the amplitude of the oscillations raises the possibility of quantum criticality. Here we discuss recently proposed mechanisms for this effect, contrasting bulk and surface scenarios. We argue that topological surface states permit us to reconcile the various data with bulk transport and spectroscopy measurements, interpreting the low temperature upturn in the quantum oscillation amplitudes as a result of surface Kondo breakdown and the high frequency oscillations as large topologically protected orbits around the X point. We discuss various predictions that can be used to test this theory.

  12. Fractionalized Fermi liquid in a Kondo-Heisenberg model

    SciTech Connect

    Tsvelik, A. M.

    2016-10-10

    The Kondo-Heisenberg model is used as a controllable tool to demonstrate the existence of a peculiar metallic state with unbroken translational symmetry where the Fermi surface volume is not controlled by the total electron density. Here, I use a nonperturbative approach where the strongest interactions are taken into account by means of exact solution, and corrections are controllable. The resulting metallic state represents a fractionalized Fermi liquid where well defined quasiparticles coexist with gapped fractionalized collective excitations, in agreement with the general requirements formulated by T. Senthil et al. [Phys. Rev. Lett. 90, 216403 (2003)]. Furthermore, the system undergoes a phase transition to an ordered phase (charge density wave or superconducting), at the transition temperature which is parametrically small in comparison to the quasiparticle Fermi energy.

  13. Interpretation of experimental results on Kondo systems with crystal field.

    PubMed

    Romero, M A; Aligia, A A; Sereni, J G; Nieva, G

    2014-01-15

    We present a simple approach to calculate the thermodynamic properties of single Kondo impurities including orbital degeneracy and crystal field effects (CFE) by extending a previous proposal by Schotte and Schotte (1975 Phys. Lett. 55A 38). Comparison with exact solutions for the specific heat of a quartet ground state split into two doublets shows deviations below 10% in the absence of CFE and a quantitative agreement for moderate or large CFE. As an application, we fit the measured specific heat of the compounds CeCu2Ge2, CePd3Si0.3, CePdAl, CePt, Yb2Pd2Sn and YbCo2Zn20. The agreement between theory and experiment is very good or excellent depending on the compound, except at very low temperatures due to the presence of magnetic correlations (not accounted for in the model).

  14. Behavior of trapped ultracold dilute Bose gases at large scattering length near a Feshbach resonance

    NASA Astrophysics Data System (ADS)

    Lekala, M. L.; Chakrabarti, B.; Rampho, G. J.; Das, T. K.; Sofianos, S. A.; Adam, R. M.

    2014-02-01

    We calculate the ground-state energy and the collective excitation frequency of trapped bosons at large scattering length interacting via the realistic two-body van der Waals potential. Our many-body method keeps two-body correlations produced by all interacting pairs. When the scattering length is small compared to the trap size and the number of bosons in the trap is of the order of a few thousands, the mean-field results are in good agreement with the many-body results. However for large particle numbers, even when the condensate is sufficiently dilute, the interatomic correlation comes into the picture. When the scattering length is quite large near the Feshbach resonance, the Bose gas becomes highly correlated. The many-body results are close to the Gross-Pitaevskii results for a small number of bosons, however, large deviations are noted in the large particle limit. We also calculate the lowest collective excitation and the interaction energy for large scattering lengths. The monopole excitation frequency exhibits a pronounced dependence on the scattering length. We also observe a universal behavior for the interaction energy at the limit of large scattering length.

  15. Electron-spin-resonance investigation of the heavy-fermion compound Ce(Cu1-xNix)2Ge2

    NASA Astrophysics Data System (ADS)

    Krug von Nidda, H.-A.; Schütz, A.; Heil, M.; Elschner, B.; Loidl, A.

    1998-06-01

    The heavy-fermion compound Ce(Cu1-xNix)2Ge2 is investigated by Gd3+ electron spin resonance (ESR) within the whole concentration range (0<=x<=1). The Kondo-lattice system exhibits an alloying-induced transition from an antiferromagnetically ordered heavy-fermion ground state (x=0) to pure Kondo-like behavior with strongly enhanced effective masses (x=1). The temperature dependence of the ESR linewidth ΔH allows one to distinguish between the different ground states. The nature of the magnetic order changes significantly from concentrations x<~0.5 to x>0.5. The ESR data provide some further experimental evidence for a transition from a local-moment type (x<0.5) to some kind of itinerant heavy-fermion band magnetism (0.5behavior is discussed for x=0.8 where the magnetism is suppressed. Our results agree very well with the 63Cu NMR spin-lattice relaxation rate 1/T1 and the dynamic structure factor S(Q,ω) obtained from inelastic neutron-scattering experiments.

  16. Distinguishing harmonic behavior of longitudinal resonant combustion in a variable geometry model rocket combustor

    NASA Astrophysics Data System (ADS)

    Hester, Sarah

    Throughout the study of high frequency combustion instability in a single element Continuously Variable Resonance Combustor (CVRC), the excitation of the fundamental longitudinal mode is closely followed by the excitation of higher harmonic modes. In an attempt to establish a heuristic relationship between the appearances of the fundamental mode and its harmonics, several unstable fixed geometry and variable geometry tests from the CVRC are analyzed through traditional Fourier-based methods and alternative signal processing methods such as wavelet analysis and Instantaneous Frequency (IF) Analysis from PC Signal Analysis. Early results led to the conclusion that traditional Fourier-based analysis provides believable and consistent results for the first three modes. However, Fourier analysis is sensitive to effects from non-sinusoidal waveforms. Further work using manufactured signals with both sinusoidal and steepfronted waveforms established that it is unclear which parts of the calculated harmonic signals are data artifacts and which are true signal. Supplementary assessment of IF Analysis and the traditional Fourier-based analysis explored the applicability of each method, the inherent data artifacts, and distinguishing behavior between the experimental data and those data artifacts. The results obtained from the IF Analysis provide good agreement with the traditional Fourier-based analysis, though one uses FIR filters and the other uses IIR filters. The validity of the results is sensitive to the settings chosen for these filters. It is shown that harmonic modal content exists in the CVRC, but it is also shown that the current results include indistinguishable Fourier artifacts. Both methods are sensitive to the sinusoidal assumption and cannot correctly interpret steep-fronted waveforms. This supplementary assessment has shown that IF Analysis is no worse than traditional Fourier-based analysis, but it fails to provide additional useful information

  17. Nonequilibrium Kondo transport through a quantum dot in a magnetic field

    NASA Astrophysics Data System (ADS)

    Smirnov, Sergey; Grifoni, Milena

    2013-07-01

    We analyze the universal transport properties of a strongly interacting quantum dot in the Kondo regime when the quantum dot is placed in an external magnetic field. The quantum dot is described by the asymmetric Anderson model with the spin degeneracy removed by the magnetic field resulting in Zeeman splitting. Using an analytical expression for the tunneling density of states found from a Keldysh effective field theory, we obtain in the whole energy range the universal differential conductance and analytically demonstrate its Fermi-liquid and logarithmic behavior at low and high energies, respectively, as a function of the magnetic field. We also show results on the zero-temperature differential conductance as a function of the bias voltage at different magnetic fields as well as results on finite-temperature effects out of equilibrium and at a finite magnetic field. The modern nonequilibrium experimental issues of the critical magnetic field, at which the zero bias maximum of the differential conductance starts to split into two maxima, as well as the distance between these maxima as a function of the magnetic field, are also addressed.

  18. Kondo effect in Co{sub x}Cu{sub 1-x} granular alloys prepared by chemical reduction method

    SciTech Connect

    Dhara, Susmita Chowdhury, Rajeswari Roy; Bandyopadhyay, Bilwadal

    2015-06-24

    Nanostructured CoCu granular alloys Co{sub x}Cu{sub 1-x} (x ≤ 0.3) have been prepared by chemical reduction method using NaBH{sub 4} as a reducing agent. Electronic transport properties are studied in the temperature range 4-300 K. Resistance exhibits a metallic behavior below room temperature and draws a minimum near 20 K in all the samples except in Co{sub 0.3}Cu{sub 0.7}. This low temperature resistivity minimum diminishes with applied magnetic field. There is also a logarithmic temperature dependence of resistivity at temperatures below 20 K. This phenomenon indicates a Kondo-like scattering mechanism involving magnetic Co impurity spin clusters in Cu host.

  19. Cancer cell uptake behavior of Au nanoring and its localized surface plasmon resonance induced cell inactivation

    NASA Astrophysics Data System (ADS)

    Chu, Che-Kuan; Tu, Yi-Chou; Chang, Yu-Wei; Chu, Chih-Ken; Chen, Shih-Yang; Chi, Ting-Ta; Kiang, Yean-Woei; Yang, Chih-Chung

    2015-02-01

    Au nanorings (NRIs), which have the localized surface plasmon resonance (LSPR) wavelength around 1058 nm, either with or without linked antibodies, are applied to SAS oral cancer cells for cell inactivation through the LSPR-induced photothermal effect when they are illuminated by a laser of 1065 nm in wavelength. Different incubation times of cells with Au NRIs are considered for observing the variations of cell uptake efficiency of Au NRI and the threshold laser intensity for cell inactivation. In each case of incubation time, the cell sample is washed for evaluating the total Au NRI number per cell adsorbed and internalized by the cells based on inductively coupled plasma mass spectrometry measurement. Also, the Au NRIs remaining on cell membrane are etched with KI/I2 solution to evaluate the internalized Au NRI number per cell. The threshold laser intensities for cell inactivation before washout, after washout, and after KI/I2 etching are calibrated from the circular area sizes of inactivated cells around the illuminated laser spot center with various laser power levels. By using Au NRIs with antibodies, the internalized Au NRI number per cell increases monotonically with incubation time up to 24 h. However, the number of Au NRI remaining on cell membrane reaches a maximum at 12 h in incubation time. The cell uptake behavior of an Au NRI without antibodies is similar to that with antibodies except that the uptake NRI number is significantly smaller and the incubation time for the maximum NRI number remaining on cell membrane is delayed to 20 h. By comparing the threshold laser intensities before and after KI/I2 etching, it is found that the Au NRIs remaining on cell membrane cause more effective cancer cell inactivation, when compared with the internalized Au NRIs.

  20. Interrogating the origin and behavior of magnetic resonance diffusion tensor scalar parameters in the myocardium

    NASA Astrophysics Data System (ADS)

    Abdullah, Osama Mahmoud

    Myocardial microstructure plays an important role in sustaining the orchestrated beating motion of the heart. Several microstructural components, including myocytes and auxiliary cells, extracellular space, and blood vessels provide the infrastructure for normal heart function, including excitation propagation, myocyte contraction, delivery of oxygen and nutrients, and removing byproduct wastes. Cardiac diseases cause deleterious changes to some or all of these microstructural components in the detrimental process of cardiac remodeling. Since heart failure is among the leading causes of death in the world, new and novel tools to noninvasively characterize heart microstructure are needed for monitoring and staging of cardiac disease. In this regards, diffusion magnetic resonance imaging (MRI) provides a promising framework to probe and quantify tissue microstructure without the need for exogenous contrast agent. As diffusion in 3-dimensional space is characterized by the diffusion tensor, MR diffusion tensor imaging (DTI) is being used to noninvasively measure anisotropic diffusion, and thus the magnitude and spatial orientation of microstructural organization of tissues, including the heart. However, even though in vivo cardiac DTI has become more clinically available, to date the origin and behavior of different microstructural components on the measured DTI signal remain to be explicitly specified. The presented studies in this work demonstrate that DTI can be used as a noninvasive and contrast-free imaging modality to characterize myocyte size and density, extracellular collagen content, and the directional magnitude of blood flow. The identified applications are expected to provide metrics to enable physicians to detect, quantify, and stage different microstructural components during progression of cardiac disease.

  1. Surface plasmon resonances behavior in visible light of non-metal perovskite oxides AgNbO{sub 3}

    SciTech Connect

    Zhou, Fei; Zhu, Jingchuan Liu, Yong; Zhao, Xiaoliang; Lai, Zhonghong

    2014-12-08

    We investigate the surface plasmon resonances (SPRs) behavior of silver niobate (AgNbO{sub 3}) experimentally and theoretically. Result shows that the localized SPRs (LSPRs) of AgNbO{sub 3} combining with its interband transitions enlarge the absorption band across the whole ultraviolet-visible range. The LSPRs behavior in visible-light is mainly ascribed to the metal-like state of silver ion and self-assembled microstructures of AgNbO{sub 3} microcrystal. The ab initio density functional theory calculations are carried out to obtain the further insight of the SPRs behaviors. Theoretical study indicates that the Ag atoms are weakly bound in the perovskite structure, leading to a metal-like state, which was the key factor to SPRs behavior of AgNbO{sub 3}.

  2. Topological Kondo Insulator (TKI) and related candidate materials: High-resolution ARPES studies

    NASA Astrophysics Data System (ADS)

    Hasan, M. Zahid

    2014-03-01

    In this talk, I plan to present ARPES (synchrotron and laser-based) studies of several mix valence and Kondo insulator phenomena in some of the rare earth heavy fermion compounds in connection to their non-trivial topology of band structures. Focus will be on SmB6 which has been predicted to be a TKI recently. By combining low-temperature and high energy-momentum resolution of the laser-based ARPES technique, for the first time, we accessed the surface electronic structure of the anomalous conductivity regime. At low T, we observe in-gap states within a 4 meV energy window of the Fermi level, which lie clearly within the bulk insulating gap. The in-gap states are found to be suppressed and eventually disappear, as the temperature is raised in approaching the coherent Kondo lattice hybridization (30 K), which proves that the in-gap states strongly depend on the existence of Kondo lattice hybridization and the effective Kondo gap, in agreement with their theoretical predicted origin of topological surface states within the Kondo insulating gap . Our Fermi mapping at the energy corresponding to these in-gap states shows distinct Fermi pockets that enclose the three Kramers' points the surface Brillouin zone, which are remarkably consistent with the theoretically predicted topological surface Fermi surface in the topological Kondo insulating phase within the level of energy resolution. The observed Fermi surface topology of the in-gap states, their temperature dependence across the transport anomaly and Kondo lattice hybridization temperatures, as well as their robustness against repeated thermal recycling, collectively not only provide a unique insight illuminating the nature of the residual conductivity anomaly but also serve as a strong experimental evidence to the predicted topological Kondo insulator phase. I also plan to present results on YbB6 and YbB12 both of which are mix valence compounds. This work is in collaboration with Madhab Neupane, N. Alidoust, S

  3. Lateral spin-orbit coupling and the Kondo effect in quantum dots

    NASA Astrophysics Data System (ADS)

    Vernek, Edson; Ngo, Anh; Ulloa, Sergio

    2010-03-01

    We present studies of the Coulomb blockade and Kondo regimes of transport of a quantum dot connected to current leads through spin-polarizing quantum point contacts (QPCs) [1]. This configuration, arising from the effect of lateral spin-orbit fields, results in spin-polarized currents even in the absence of external magnetic fields and greatly affects the correlations in the dot. Using an equation-of-motion technique and numerical renormalization group calculations we obtain the conductance and spin polarization for this system under different parameter regimes. Our results show that both the Coulomb blockade and Kondo regimes exhibit non-zero spin-polarized conductance. We analyze the role that the spin-dependent tunneling amplitudes of the QPC play in determining the charge and net magnetic moment in the dot. We find that the Kondo regime exhibits a strongly dependent Kondo temperature on the QPC polarizability. These effects, controllable by lateral gate voltages, may provide a new approach for exploring Kondo correlations, as well as possible spin devices. Supported by NSF DMR-MWN and PIRE. [1] P. Debray et al., Nature Nanotech. 4, 759 (2009).

  4. Orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films

    PubMed Central

    Zhu, L. J.; Nie, S. H.; Xiong, P.; Schlottmann, P.; Zhao, J. H.

    2016-01-01

    The orbital two-channel Kondo effect displaying exotic non-Fermi liquid behaviour arises in the intricate scenario of two conduction electrons compensating a pseudo-spin-1/2 impurity of two-level system. Despite extensive efforts for several decades, no material system has been clearly identified to exhibit all three transport regimes characteristic of the two-channel Kondo effect in the same sample, leaving the interpretation of the experimental results a subject of debate. Here we present a transport study suggestive of a robust orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films, as evidenced by a magnetic field-independent resistivity upturn with a clear transition from logarithmic- to square-root temperature dependence and deviation from it in three distinct temperature regimes. Our results also provide an experimental indication of the presence of two-channel Kondo physics in a ferromagnet, pointing to considerable robustness of the orbital two-channel Kondo effect even in the presence of spin polarization of the conduction electrons. PMID:26905518

  5. Kondo effect in a quantum wire with spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    de Sousa, G. R.; Silva, Joelson F.; Vernek, E.

    2016-09-01

    The influence of spin-orbit interactions on the Kondo effect has been under debate recently. Studies conducted recently on a system composed of an Anderson impurity on a two-dimensional electron gas with a Rashba spin orbit have shown that it can enhance or suppress the Kondo temperature (TK), depending on the relative energy level position of the impurity with respect to the particle-hole symmetric point. Here, we investigate a system composed of a single Anderson impurity, side coupled to a quantum wire with spin-orbit coupling (SOC). We derive an effective Hamiltonian in which the Kondo coupling is modified by the SOC. In addition, the Hamiltonian contains two other scattering terms, the so-called Dzyaloshinskii-Moriya interaction, known to appear in these systems, and another one describing processes similar to the Elliott-Yafet scattering mechanisms. By performing a renormalization group analysis on the effective Hamiltonian, we find that the correction on the Kondo coupling due to the SOC favors the enhancement of the Kondo temperature even in the particle-hole symmetric point of the Anderson model, agreeing with the numerical renormalization group results. Moreover, away from the particle-hole symmetric point, TK always increases with the SOC, accordingly with a previous renormalization group analysis.

  6. Ferromagnetism in the Kondo-lattice compound CePd2P2.

    PubMed

    Tran, Vinh Hung; Bukowski, Zbigniew

    2014-06-25

    We report physical properties of CePd2P2 crystallizing in the tetragonal ThCr2Si2-type structure (space group I4/mmm). Dc-magnetic susceptibility, magnetization, specific heat, electrical resistivity and magnetoresistance measurements establish a ferromagnetic ordering below the Curie temperature TC = 28.4 ± 0.2 K. Critical analysis of isothermal and isofield magnetization yields critical exponents of β = 0.405 ± 0.005, γ = 1.11 ± 0.05 and δ = 3.74 ± 0.04. The ordered state is characterized by saturation moment Ms ∼ 0.98μB and magnon energy gap Δ/kB ∼25–35 K. The studied properties reflect a competing influence of the Kondo and crystalline electric field (CEF) interactions. The strength of the Kondo effect is assigned by a low-temperature Kondo scale TK ∼19 ± 10 K and a high-temperature Kondo scale TK ~ H 117 } 10 K. A model of the inelastic scattering of the conduction electrons with an exchanged CEF energy ΔCEF was applied to the magnetic resistivity. An average value ΔCEF = 260 ± 30 K is consistent in the relationships with TK and TK H. We argue that the CePd2P2 compound appears to be a new ferromagnetic Kondo-lattice among the Ce-based intermetallics.

  7. Orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films

    DOE PAGES

    Zhu, L. J.; Nie, S. H.; Xiong, P.; ...

    2016-02-24

    The orbital two-channel Kondo effect displaying exotic non-Fermi liquid behaviour arises in the intricate scenario of two conduction electrons compensating a pseudo-spin-1/2 impurity of two-level system. Despite extensive efforts for several decades, no material system has been clearly identified to exhibit all three transport regimes characteristic of the two-channel Kondo effect in the same sample, leaving the interpretation of the experimental results a subject of debate. Here we present a transport study suggestive of a robust orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films, as evidenced by a magnetic field-independent resistivity upturn with a clear transition from logarithmic- tomore » square-root temperature dependence and deviation from it in three distinct temperature regimes. Lastly, our results also provide an experimental indication of the presence of two-channel Kondo physics in a ferromagnet, pointing to considerable robustness of the orbital two-channel Kondo effect even in the presence of spin polarization of the conduction electrons.« less

  8. Quantum interference and Kondo effects in an Aharonov-Bohm-Casher interferometer containing a laterally coupled double quantum dot

    NASA Astrophysics Data System (ADS)

    Kubo, T.; Tokura, Y.; Tarucha, S.

    2010-01-01

    We theoretically investigate spin-dependent electron transport through an Aharonov-Bohm-Casher interferometer containing a laterally coupled double quantum dot. In particular, we numerically calculate the Aharonov-Bohm and Aharonov-Casher oscillations of the linear conductance in the Kondo regime. We show that the AC oscillation in the Kondo regime deviates from the sinusoidal form.

  9. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: Electric-Current-Induced Heat Generation in Kondo Regime

    NASA Astrophysics Data System (ADS)

    Chen, Qiao; Zhang, Ya-Min

    2010-07-01

    Using the nonequilibrium Green's function technique, we investigate the current induced heat generation in Kondo regime. The Kondo effect influences the heat generation significantly. In the curve of heat generation versus the bias, a negative differential of the heat generation is exhibited. The symmetry of the heat generation is destroyed by the strong electron-electron interaction and the electron-phonon interaction.

  10. X-boson cumulant approach to the topological Kondo insulators

    NASA Astrophysics Data System (ADS)

    Ramos, E.; Franco, R.; Silva-Valencia, J.; Foglio, M. E.; Figueira, M. S.

    2014-12-01

    In this work we present a generalization of our previous work of the X-boson approach to the periodic Anderson model (PAM), adequate to study a novel class of intermetallic 4f and 5f orbitals materials: the topological Kondo insulators, whose paradigmatic material is the compound SmB6. For simplicity, we consider a version of the PAM on a 2D square lattice, adequate to describe Ce-based compounds in two dimensions. The starting point of the model is the 4f - Ce ions orbitals, with J = 5/2 multiplet, in the presence of spin-orbit coupling. Our technique works well for all of the parameters of the model and avoids the unwanted phase transitions of the slave boson mean field theory. We present a critical comparison of our results with those of the usual slave boson method, that has been intensively used to describe this class of materials. We also obtain a new valence first order transition which we attribute to the vec k dependence of the hybridization.

  11. First-principles study of the Kondo physics of a single Pu impurity in a Th host

    SciTech Connect

    Zhu, Jian -Xin; Albers, R. C.; Haule, K.; Wills, J. M.

    2015-04-23

    Based on its condensed-matter properties, crystal structure, and metallurgy, which includes a phase diagram with six allotropic phases, plutonium is one of the most complicated pure elements in its solid state. Its anomalous properties, which are indicative of a very strongly correlated state, are related to its special position in the periodic table, which is at the boundary between the light actinides that have itinerant 5f electrons and the heavy actinides that have localized 5f electrons. As a foundational study to probe the role of local electronic correlations in Pu, we use the local-density approximation together with a continuous-time quantum Monte Carlo simulation to investigate the electronic structure of a single Pu atom that is either substitutionally embedded in the bulk and or adsorbed on the surface of a Th host. This is a simpler case than the solid phases of Pu metal. With the Pu impurity atom we have found a Kondo resonance peak, which is an important signature of electronic correlations, in the local density of states around the Fermi energy. We show that the peak width of this resonance is narrower for Pu atoms at the surface of Th than for those in the bulk due to a weakened Pu - 5f hybridization with the ligands at the surface.

  12. First-principles study of the Kondo physics of a single Pu impurity in a Th host

    DOE PAGES

    Zhu, Jian -Xin; Albers, R. C.; Haule, K.; ...

    2015-04-23

    Based on its condensed-matter properties, crystal structure, and metallurgy, which includes a phase diagram with six allotropic phases, plutonium is one of the most complicated pure elements in its solid state. Its anomalous properties, which are indicative of a very strongly correlated state, are related to its special position in the periodic table, which is at the boundary between the light actinides that have itinerant 5f electrons and the heavy actinides that have localized 5f electrons. As a foundational study to probe the role of local electronic correlations in Pu, we use the local-density approximation together with a continuous-time quantummore » Monte Carlo simulation to investigate the electronic structure of a single Pu atom that is either substitutionally embedded in the bulk and or adsorbed on the surface of a Th host. This is a simpler case than the solid phases of Pu metal. With the Pu impurity atom we have found a Kondo resonance peak, which is an important signature of electronic correlations, in the local density of states around the Fermi energy. We show that the peak width of this resonance is narrower for Pu atoms at the surface of Th than for those in the bulk due to a weakened Pu - 5f hybridization with the ligands at the surface.« less

  13. Spin relaxation and the Kondo effect in transition metal dichalcogenide monolayers.

    PubMed

    Rostami, Habib; Moghaddam, Ali G; Asgari, Reza

    2016-12-21

    We investigate the spin relaxation and Kondo resistivity caused by magnetic impurities in doped transition metal dichalcogenide monolayers. We show that momentum and spin relaxation times, due to the exchange interaction by magnetic impurities, are much longer when the Fermi level is inside the spin-split region of the valence band. In contrast to the spin relaxation, we find that the dependence of Kondo temperature T K on the doping is not strongly affected by the spin-orbit induced splitting, although only one of the spin species are present at each valley. This result, which is obtained using both perturbation theory and the poor man's scaling methods, originates from the intervalley spin-flip scattering in the spin-split region. We further demonstrate the decline in the conductivity with temperatures close to T K, which can vary with the doping. Our findings reveal the qualitative difference with the Kondo physics in conventional metallic systems and other Dirac materials.

  14. Spin relaxation and the Kondo effect in transition metal dichalcogenide monolayers

    NASA Astrophysics Data System (ADS)

    Rostami, Habib; Moghaddam, Ali G.; Asgari, Reza

    2016-12-01

    We investigate the spin relaxation and Kondo resistivity caused by magnetic impurities in doped transition metal dichalcogenide monolayers. We show that momentum and spin relaxation times, due to the exchange interaction by magnetic impurities, are much longer when the Fermi level is inside the spin-split region of the valence band. In contrast to the spin relaxation, we find that the dependence of Kondo temperature T K on the doping is not strongly affected by the spin-orbit induced splitting, although only one of the spin species are present at each valley. This result, which is obtained using both perturbation theory and the poor man’s scaling methods, originates from the intervalley spin-flip scattering in the spin-split region. We further demonstrate the decline in the conductivity with temperatures close to T K, which can vary with the doping. Our findings reveal the qualitative difference with the Kondo physics in conventional metallic systems and other Dirac materials.

  15. Understanding the Josephson current through a Kondo-correlated quantum dot.

    PubMed

    Luitz, D J; Assaad, F F; Novotný, T; Karrasch, C; Meden, V

    2012-06-01

    We study the Josephson current 0-π transition of a quantum dot tuned to the Kondo regime. The physics can be quantitatively captured by the numerically exact continuous time quantum Monte Carlo method applied to the single-impurity Anderson model with Bardeen-Cooper-Schrieffer superconducting leads. For a comparison to an experiment, the tunnel couplings are determined by fitting the normal-state linear conductance. Excellent agreement for the dependence of the critical Josephson current on the level energy is achieved. For increased tunnel couplings the Kondo scale becomes comparable to the superconducting gap, and the regime of the strongest competition between superconductivity and Kondo correlations is reached; we predict the gate voltage dependence of the critical current in this regime.

  16. Displacement front behavior of near miscible CO2 flooding in decane saturated synthetic sandstone cores revealed by magnetic resonance imaging.

    PubMed

    Liu, Yu; Teng, Ying; Jiang, Lanlan; Zhao, Jiafei; Zhang, Yi; Wang, Dayong; Song, Yongchen

    2017-04-01

    It is of great importance to study the CO2-oil two-phase flow characteristic and displacement front behavior in porous media, for understanding the mechanisms of CO2 enhanced oil recovery. In this work, we carried out near miscible CO2 flooding experiments in decane saturated synthetic sandstone cores to investigate the displacement front characteristic by using magnetic resonance imaging technique. Experiments were done in three consolidated sandstone cores with the permeabilities ranging from 80 to 450mD. The oil saturation maps and the overall oil saturation during CO2 injections were obtained from the intensity of magnetic resonance imaging. Finally the parameters of the piston-like displacement fronts, including the front velocity and the front geometry factor (the length to width ratio) were analyzed. Experimental results showed that the near miscible vertical upward displacement is instable above the minimum miscible pressure in the synthetic sandstone cores. However, low permeability can restrain the instability to some extent.

  17. Kondo effect in transport through Aharonov-Bohm and Aharonov-Casher interferometers

    NASA Astrophysics Data System (ADS)

    Lobos, A. M.; Aligia, A. A.

    2009-10-01

    We derive the extension of the Hubbard model to include Rashba spin-orbit coupling that correctly describes Aharonov-Bohm and Aharonov-Casher phases in a ring under applied magnetic and electric fields. When the ring is connected to conducting leads, we develop a formalism that is able to describe both, Kondo and interference effects. We find that in the Kondo regime, the spin-orbit coupling reduces strongly the conductance from the unitary limit. This effect in combination with the magnetic flux, can be used to produce spin polarized carriers.

  18. Gap formation and phase transition of the anisotropic Kondo necklace model: Density matrix renormalization group analysis

    NASA Astrophysics Data System (ADS)

    Mendoza-Arenas, J. J.; Franco, R.; Silva-Valencia, J.

    2010-01-01

    We analyze the one-dimensional Kondo necklace model, at zero temperature, with an anisotropy parameter η in the interaction of the conduction chain, by means of the density matrix renormalization group. We calculate the energy gap and estimate the quantum critical points that separate a Kondo singlet state from an antiferromagnetic state, assuming a Kosterlitz-Thouless tendency. We also observe the correlation functions and the structure factors that support our critical points. The resulting phase diagram is presented and compared to that reported previously using Lanczos calculations. It is shown that the quantum critical points vary very slowly with η , but when η approaches zero, they drop abruptly.

  19. Spin-orbit interactions in a helical Luttinger liquid with a Kondo impurity

    NASA Astrophysics Data System (ADS)

    Eriksson, Erik

    2013-03-01

    We study the transport properties of a helical Luttinger liquid with a Kondo impurity and spin-orbit interactions. Such a system, which may be realized at the edge of a quantum spin Hall insulator with a gate-induced electric field, provides a mechanism to electrically control the conductance. A Rashba spin-orbit interaction may even change the nature of the Kondo screening [Eriksson et al., Phys. Rev. B 86, 161103(R) (2012)]. Considering other types of spin-orbit interactions, together with an extended non-equilibrium analysis, we further improve the understanding of these phenomena.

  20. Observation of the Kondo effect in a spin-3/2 hole quantum dot

    SciTech Connect

    Klochan, O.; Micolich, A. P.; Hamilton, A. R.; Trunov, K.; Reuter, D.; Wieck, A. D.

    2013-12-04

    We report the observation of the Kondo effect in a spin-3/2 hole quantum dot formed near pinch-off in a GaAs quantum wire. We clearly observe two distinctive hallmarks of quantum dot Kondo physics. First, the zero-bias peak in the differential conductance splits an in-plane magnetic field and the splitting is independent of gate voltage. Second, the splitting rate is twice as large as that for the lowest one-dimensional subband. We show that the Zeeman splitting of the zero-bias peak is highly anisotropic and attribute this to the strong spin-orbit interaction for holes in GaAs.

  1. Magnetoresistance in the Spin-Orbit Kondo State of Elemental Bismuth

    PubMed Central

    Craco, Luis; Leoni, Stefano

    2015-01-01

    Materials with strong spin-orbit coupling, which competes with other particle-particle interactions and external perturbations, offer a promising route to explore novel phases of quantum matter. Using LDA + DMFT we reveal the complex interplay between local, multi-orbital Coulomb and spin-orbit interaction in elemental bismuth. Our theory quantifies the role played by collective dynamical fluctuations in the spin-orbit Kondo state. The correlated electronic structure we derive is promising in the sense that it leads to results that might explain why moderate magnetic fields can generate Dirac valleys and directional-selective magnetoresistance responses within spin-orbit Kondo metals. PMID:26358556

  2. Can functional magnetic resonance imaging studies help with the optimization of health messaging for lifestyle behavior change? A systematic review.

    PubMed

    Whelan, Maxine E; Morgan, Paul S; Sherar, Lauren B; Orme, Mark W; Esliger, Dale W

    2017-02-15

    Unhealthy behaviors, including smoking, poor nutrition, excessive alcohol consumption, physical inactivity and sedentary lifestyles, are global risk factors for non-communicable diseases and premature death. Functional magnetic resonance imaging (fMRI) offers a unique approach to optimize health messages by examining how the brain responds to information relating to health. Our aim was to systematically review fMRI studies that have investigated variations in brain activation in response to health messages relating to (i) smoking; (ii) alcohol consumption; (iii) physical activity; (iv) diet; and (v) sedentary behavior. The electronic databases used were Medline/PubMed, Web of Science (Core Collection), PsychINFO, SPORTDiscuss, Cochrane Library and Open Grey. Studies were included if they investigated subjects aged ≥10years and were published before January 2017. Of the 13,836 studies identified in the database search, 18 studies (smoking k=15; diet k=2; physical activity/sedentary behavior k=1) were included in the review. The prefrontal cortex was activated in seven (47%) of the smoking-related studies and the physical activity study. Results suggest that activation of the ventromedial, dorsolateral and medial prefrontal cortex regions were predictive of subsequent behavior change following exposure to aversive anti-smoking stimuli. Studies investigating the neurological responses to anti-smoking material were most abundant. Of note, the prefrontal cortex and amygdala were most commonly activated in response to health messages across lifestyle behaviors. The review highlights an important disparity between research focusing on different lifestyle behaviors. Insights from smoking literature suggest fMRI may help to optimize health messaging in relation to other lifestyle behaviors.

  3. Magnetic moments and non-Fermi-liquid behavior in quasicrystals

    NASA Astrophysics Data System (ADS)

    Andrade, Eric

    Motivated by the intrinsic non-Fermi-liquid behavior observed in the heavy-fermion quasicrystal Au51Al34Yb15, we study the low-temperature behavior of dilute magnetic impurities placed in metallic quasicrystals. We find that a large fraction of the magnetic moments are not quenched down to very low temperatures, leading to a power-law distribution of Kondo temperatures, accompanied by a non-Fermi-liquid behavior, in a remarkable similarity to the Kondo-disorder scenario found in disordered heavy-fermion metals. This work was supported by FAPESP (Brazil) Grant No. 2013/00681-8.

  4. If It's Resonance, What is Resonating?

    ERIC Educational Resources Information Center

    Kerber, Robert C.

    2006-01-01

    The phenomenon under the name "resonance," which, is based on the mathematical analogy between mechanical resonance and the behavior of wave functions in quantum mechanical exchange phenomena was described. The resonating system does not have a structure intermediate between those involved in the resonance, but instead a structure which is further…

  5. Nonlinear dynamic behaviors of clamped laminated shallow shells with one-to-one internal resonance

    NASA Astrophysics Data System (ADS)

    Abe, Akira; Kobayashi, Yukinori; Yamada, Gen

    2007-07-01

    This paper investigates one-to-one internal resonance of laminated shallow shells with rigidly clamped edges. It is assumed that the natural frequencies ω2 and ω3 of two asymmetric (second and third) vibration modes have the relationship ω2≈ ω3. The displacements are expressed by using eigenvectors for linear vibration modes calculated by the Ritz method. Applying Galerkin's procedure to the equation of motion, nonlinear differential equations are derived. By considering the first vibration mode in addition to the two asymmetric vibration modes, quadratic nonlinear terms expressing the interaction between the asymmetric and the first modes appear in the differential equations. Shooting method is used to obtain the steady-state response when the driving frequency Ω is near ω2. The dynamic characteristics of the shells with the internal resonance are discussed.

  6. Influence of the Basset force on the resonant behavior of an oscillator with fluctuating frequency

    SciTech Connect

    Rekker, A. Mankin, R.

    2015-10-28

    The influence of hydrodynamic interactions, such as Stokes and Basset forces, on the dynamics of a harmonically trapped Brownian tracer is considered. A generalized Langevin equation is used to describe the tracer’s response to an external periodic force and to dichotomous fluctuations of the stiffness of the trapping potential. Relying on the Shapiro-Loginov formula, exact expressions for the complex susceptibility and for the response function are presented. On the basis of these exact formulas, it is demonstrated that interplay of a multiplicative colored noise and the Basset force induced memory effects can generate a variety of cooperation effects, such as multiresonance versus the driving frequency, as well as stochastic resonance versus noise parameters. In particular, in certain parameter regions the response function exhibits a resonance-like enhancement at intermediate values of the intensity of the Basset force. Conditions for the appearance of these effects are also discussed.

  7. Environment-modulated Kondo phenomena in FePc/Au(111) adsorption systems

    NASA Astrophysics Data System (ADS)

    Wang, Yu; Zheng, Xiao; Yang, Jinlong

    2016-03-01

    Recent scanning tunneling microscopy experiments on electron transport through iron(II) phthalocyanine (FePc) molecules adsorbed on the Au(111) surface have revealed that the measured Kondo conductance signature depends strongly on the specific adsorption site. To understand the physical origin of experimental observations, particularly the variation of Kondo features with the molecular adsorption site, we employ a combined density functional theory (DFT) and hierarchical equations of motion (HEOM) approach to investigate the electronic structure and Kondo correlation in FePc/Au(111) composite systems. The calculation results indicate that, for the on-top adsorption configuration, the two degenerate spin-unpaired dπ orbitals on the Fe center are coupled indirectly through substrate band states, leading to the Fano-like antiresonance line shape in the d I /d V spectra, while for the bridge adsorption configuration, the environment-induced couplings are largely suppressed because of the two different spin-unpaired d orbitals. Therefore, our work suggests that the environment-induced coupling as an essential physical factor could greatly influence the Fano-Kondo features in magnetic molecule/metal composites, and the crucial role of local orbital degeneracy and symmetry is discovered. These findings provide important insights into the electron correlation effects in complex solid-state systems. The usefulness and practicality of the combined DFT+HEOM method is also highlighted.

  8. Strong spin Seebeck effect in Kondo T-shaped double quantum dots.

    PubMed

    Wójcik, K P; Weymann, I

    2017-02-08

    We investigate, taking a theoretical approach, the thermoelectric and spin thermoelectric properties of a T-shaped double quantum dot strongly coupled to two ferromagnetic leads, focusing on the transport regime in which the system exhibits the two-stage Kondo effect. We study the dependence of the (spin) Seebeck coefficient, the corresponding power factor and the figure of merit on temperature, leads' spin polarization and dot level position. We show that the thermal conductance fulfills a modified Wiedemann-Franz law, also in the regime of suppression of subsequent stages of the Kondo effect by the exchange field resulting from the presence of ferromagnets. Moreover, we demonstrate that the spin thermopower is enhanced at temperatures corresponding to the second stage of Kondo screening. Very interestingly, the spin-thermoelectric response of the system is found to be highly sensitive to the spin polarization of the leads. In some cases spin polarization of the order of 1% is sufficient for a strong spin Seebeck effect to occur. This is explained as a consequence of the interplay between the two-stage Kondo effect and the exchange field induced in the double quantum dot. Due to the possibility of tuning the exchange field by the choice of gate voltage, the spin thermopower may also be tuned to be maximal for desired spin polarization of the leads. All calculations are performed with the aid of the numerical renormalization group technique.

  9. Spin relaxation through Kondo scattering in Cu/Py lateral spin valves

    NASA Astrophysics Data System (ADS)

    Batley, J. T.; Rosaond, M. C.; Ali, M.; Linfield, E. H.; Burnell, G.; Hickey, B. J.

    Within non-magnetic metals it is reasonable to expect the Elliot-Yafet mechanism to govern spin-relaxation and thus the temperature dependence of the spin diffusion length might be inversely proportional to resistivity. However, in lateral spin valves, measurements have found that at low temperatures the spin diffusion length unexpectedly decreases. We have fabricated lateral spin valves from Cu with different concentrations of magnetic impurities. Through temperature dependent charge and spin transport measurements we present clear evidence linking the presence of the Kondo effect within Cu to the suppression of the spin diffusion length below 30 K. We have calculated the spin-relaxation rate and isolated the contribution from magnetic impurities. At very low temperatures electron-electron interactions play a more prominent role in the Kondo effect. Well below the Kondo temperature a strong-coupling regime exists, where the moments become screened and the magnetic dephasing rate is reduced. We also investigate the effect of this low temperature regime (>1 K) on a pure spin current. This work shows the dominant role of Kondo scattering, even in low concentrations of order 1 ppm, within pure spin transport.

  10. Analytical expression of Kondo temperature in quantum dot embedded in Aharonov-Bohm ring

    PubMed Central

    2011-01-01

    We theoretically study the Kondo effect in a quantum dot embedded in an Aharonov-Bohm ring, using the "poor man's" scaling method. Analytical expressions of the Kondo temperature TK are given as a function of magnetic flux Φ penetrating the ring. In this Kondo problem, there are two characteristic lengths, Lc=ℏvF∕|ε˜0| and LK = ħvF = TK, where vF is the Fermi velocity and ε˜0 is the renormalized energy level in the quantum dot. The former is the screening length of the charge fluctuation and the latter is that of the spin fluctuation, i.e., size of Kondo screening cloud. We obtain diferent expressions of TK(Φ) for (i) Lc ≪ LK ≪ L, (ii) Lc ≪ L ≪ LK, and (iii) L ≪ Lc ≪ LK, where L is the size of the ring. TK is remarkably modulated by Φ in cases (ii) and (iii), whereas it hardly depends on Φ in case (i). PACS numbers: PMID:22112300

  11. Strong spin Seebeck effect in Kondo T-shaped double quantum dots

    NASA Astrophysics Data System (ADS)

    Wójcik, K. P.; Weymann, I.

    2017-02-01

    We investigate, taking a theoretical approach, the thermoelectric and spin thermoelectric properties of a T-shaped double quantum dot strongly coupled to two ferromagnetic leads, focusing on the transport regime in which the system exhibits the two-stage Kondo effect. We study the dependence of the (spin) Seebeck coefficient, the corresponding power factor and the figure of merit on temperature, leads’ spin polarization and dot level position. We show that the thermal conductance fulfills a modified Wiedemann-Franz law, also in the regime of suppression of subsequent stages of the Kondo effect by the exchange field resulting from the presence of ferromagnets. Moreover, we demonstrate that the spin thermopower is enhanced at temperatures corresponding to the second stage of Kondo screening. Very interestingly, the spin-thermoelectric response of the system is found to be highly sensitive to the spin polarization of the leads. In some cases spin polarization of the order of 1% is sufficient for a strong spin Seebeck effect to occur. This is explained as a consequence of the interplay between the two-stage Kondo effect and the exchange field induced in the double quantum dot. Due to the possibility of tuning the exchange field by the choice of gate voltage, the spin thermopower may also be tuned to be maximal for desired spin polarization of the leads. All calculations are performed with the aid of the numerical renormalization group technique.

  12. Analytical expression of Kondo temperature in quantum dot embedded in Aharonov-Bohm ring.

    PubMed

    Yoshii, Ryosuke; Eto, Mikio

    2011-11-23

    We theoretically study the Kondo effect in a quantum dot embedded in an Aharonov-Bohm ring, using the "poor man's" scaling method. Analytical expressions of the Kondo temperature TK are given as a function of magnetic flux Φ penetrating the ring. In this Kondo problem, there are two characteristic lengths, Lc=ℏvF∕|ε̃0| and LK = ħvF = TK, where vF is the Fermi velocity and ε̃0 is the renormalized energy level in the quantum dot. The former is the screening length of the charge fluctuation and the latter is that of the spin fluctuation, i.e., size of Kondo screening cloud. We obtain diferent expressions of TK(Φ) for (i) Lc ≪ LK ≪ L, (ii) Lc ≪ L ≪ LK, and (iii) L ≪ Lc ≪ LK, where L is the size of the ring. TK is remarkably modulated by Φ in cases (ii) and (iii), whereas it hardly depends on Φ in case (i).PACS numbers:

  13. A theoretical study of the spin glass-Kondo-magnetic disordered alloys in the presence of a random field

    NASA Astrophysics Data System (ADS)

    Magalhaes, S. G.; Zimmer, F. M.; Coqblin, B.

    2012-12-01

    We study here the influence of a random applied magnetic field on the competition between the Kondo effect, the spin glass phase and a ferromagnetic order in disordered cerium systems such as CeNi1-xCux. The model used here takes an intrasite Kondo coupling and an intersite random coupling; both the intersite random coupling and the random magnetic field are described within the Sherrington-Kirkpatrick model and the one-step replica symmetry breaking procedure is also used here. We present phase diagrams giving Temperature versus the Kondo exchange parameter and the random magnetic field makes decrease particularly the importance of the spin glass and ferromagnetic phases.

  14. Antiferromagnetic Kondo lattice in the layered compound CePd1–xBi₂ and comparison to the superconductor LaPd1–xBi₂

    DOE PAGES

    Han, Fei; Wan, Xiangang; Phelan, Daniel; ...

    2015-07-13

    The layered compound CePd1–xBi₂ with the tetragonal ZrCuSi₂-type structure was obtained from excess Bi flux. Magnetic susceptibility data of CePd1–xBi₂ show an antiferromagnetic ordering below 6 K and are anisotropic along the c axis and the ab plane. The anisotropy is attributed to crystal-electric-field (CEF) effects and a CEF model which is able to describe the susceptibility data is given. An enhanced Sommerfeld coefficient γ of 0.191 J mol Ce⁻¹ K⁻² obtained from specific-heat measurement suggests a moderate Kondo effect in CePd1–xBi₂. Other than the antiferromagnetic peak at 6 K, the resistivity curve shows a shoulderlike behavior around 75 Kmore » which could be attributed to the interplay between Kondo and CEF effects. Magnetoresistance and Hall-effect measurements suggest that the interplay reconstructs the Fermi-surface topology of CePd1–xBi₂ around 75 K. Electronic structure calculations reveal that the Pd vacancies are important to the magnetic structure and enhance the CEF effects which quench the orbital moment of Ce at low temperatures.« less

  15. Double threshold behavior in a resonance-controlled ZnO random laser

    NASA Astrophysics Data System (ADS)

    Niyuki, Ryo; Fujiwara, Hideki; Nakamura, Toshihiro; Ishikawa, Yoshie; Koshizaki, Naoto; Tsuji, Takeshi; Sasaki, Keiji

    2017-03-01

    We observed unusual lasing characteristics, such as double thresholds and blue-shift of lasing peak, in a resonance-controlled ZnO random laser. From the analysis of lasing threshold carrier density, we found that the lasing at 1st and 2nd thresholds possibly arises from different mechanisms; the lasing at 1st threshold involves exciton recombination, whereas the lasing at 2nd threshold is caused by electron-hole plasma recombination, which is the typical origin of conventional random lasers. These phenomena are very similar to the transition from polariton lasing to photon lasing observed in a well-defined cavity laser.

  16. Bragg resonance behavior of the neutron refractive index and crystal acceleration effect

    NASA Astrophysics Data System (ADS)

    Braginetz, Yu. P.; Berdnikov, Ya. A.; Fedorov, V. V.; Kuznetsov, I. A.; Lasitsa, M. V.; Semenikhin, S. Yu.; Vezhlev, E. O.; Voronin, V. V.

    2016-09-01

    The energy dependence of neutron refraction index in a perfect crystal for neutron energy, close to the Bragg ones, was studied. The resonance shape of this dependence with approximately the Darwin width was found. As a result, the value of deviation from the exact Bragg condition can change during the neutron time of flight through the accelerated crystal and so the refraction index and the velocity of outgoing neutron can change as well. Such new mechanism of neutron acceleration in the accelerating perfect crystal was proposed and found experimentally. This mechanism is march more effective then known one concerning with the neutron acceleration in the accelerating usual media.

  17. Cyclotron dynamics of a Kondo singlet in a spin-orbit-coupled alkaline-earth-metal atomic gas

    NASA Astrophysics Data System (ADS)

    Jiang, Bo-Nan; Lv, Hao; Wang, Wen-Li; Du, Juan; Qian, Jun; Wang, Yu-Zhu

    2014-11-01

    We propose a scheme to investigate the interplay between the Kondo-exchange interaction and the quantum spin Hall effect with ultracold fermionic alkaline-earth-metal atoms trapped in two-dimensional optical lattices using ultracold collision and laser-assisted tunneling. In the strong Kondo-coupling regime, although the loop trajectory of the mobile atom disappears, collective dynamics of an atom pair in two clock states can exhibit an unexpected spin-dependent cyclotron orbit in a plaquette, realizing the quantum spin Hall effect of the Kondo singlet. We demonstrate that the collective cyclotron dynamics of the spin-zero Kondo singlet is governed by an effective Harper-Hofstadter model in addition to second-order diagonal tunneling.

  18. Genome sequence of Frateuria aurantia type strain (Kondo 67(T)), a xanthomonade isolated from Lilium auratium Lindl.

    SciTech Connect

    Anderson, Iain; Teshima, Hazuki; Nolan, Matt; Lapidus, Alla L.; Tice, Hope; Glavina Del Rio, Tijana; Cheng, Jan-Fang; Han, Cliff; Tapia, Roxanne; Goodwin, Lynne A.; Pitluck, Sam; Liolios, Konstantinos; Mavromatis, K; Pagani, Ioanna; Ivanova, N; Mikhailova, Natalia; Pati, Amrita; Chen, Amy; Palaniappan, Krishna; Land, Miriam L; Rohde, Manfred; Lang, Elke; Detter, J. Chris; Goker, Markus; Woyke, Tanja; Bristow, James; Eisen, Jonathan; Markowitz, Victor; Hugenholtz, Philip; Kyrpides, Nikos C; Klenk, Hans-Peter

    2013-01-01

    rateuria aurantia (ex Kondo and Ameyama 1958) Swings et al. 1980 is a member of the bispecific genus Frateuria in the family Xanthomonadaceae, which is already heavily targeted for non-type strain genome sequencing. Strain Kondo 67(T) was initially (1958) identified as a member of 'Acetobacter aurantius', a name that was not considered for the approved list. Kondo 67(T) was therefore later designated as the type strain of the newly proposed acetogenic species Frateuria aurantia. The strain is of interest because of its triterpenoids (hopane family). F. aurantia Kondo 67(T) is the first member of the genus Frateura whose genome sequence has been deciphered, and here we describe the features of this organism, together with the complete genome sequence and annotation. The 3,603,458-bp long chromosome with its 3,200 protein-coding and 88 RNA genes is a part of the Genomic Encyclopedia of Bacteria and Archaea project.

  19. Origin of bulk quantum oscillations in the bulk Kondo insulating ground state of SmB6

    NASA Astrophysics Data System (ADS)

    Sebastian, Suchitra; Tan, B. S.; Hsu, Y.-T.; Zeng, B.; Ciomaga Hatnean, M.; Harrison, N.; Zhu, Z.; Hartstein, M.; Kiourlappou, M.; Srivastava, M.; Johannes, M. D.; Murphy, T. P.; Park, J.-H.; Balicas, L.; Shitsevalova, N.; Lonzarich, G. G.; Balakrishnan, G.

    I will discuss our recent observation of quantum oscillations corresponding to a bulk Fermi surface in the Kondo insulator SmB6, and consider their possible origin. New complementary experimental results will be presented which raise the interesting question of whether the underlying ground state corresponds to a novel Kondo regime in which the spin channel is gapless while the charge channel is gapped.

  20. Heavy-Fermion Valence-Bond Liquids in Ultracold Atoms: Cooperation of the Kondo Effect and Geometric Frustration.

    PubMed

    Isaev, L; Rey, A M

    2015-10-16

    We analyze a microscopic mechanism behind the coexistence of a heavy Fermi liquid and geometric frustration in Kondo lattices. We consider a geometrically frustrated periodic Anderson model and demonstrate how orbital fluctuations lead to a Kondo-screened phase in the limit of extreme strong frustration when only local singlet states participate in the low-energy physics. We also propose a setup to realize and study this exotic state with SU(3)-symmetric alkaline-earth cold atoms.

  1. ESR (electron spin resonance)-determined osmotic behavior of bull spermatozoa

    SciTech Connect

    Du, J.; Kleinhans, F.W.; Spitzer, V.J.; Critser, J.K. . Dept. of Medical Research); Horstman, L. . School of Veterinary Medicine); Mazur, P. )

    1990-01-01

    Our laboratories are pursuing a fundamental approach to the problems of semen cryopreservation. For many cell types (human red cells, yeast, HeLa) it has been demonstrated that there is an optimum cooling rate for cryopreservation. Faster rates allow insufficient time for cell dehydration and result in intracellular ice formation and cell death. It is possible to predict this optimal rate provided that the cell acts as an ideal osmometer and several other cell parameters are known such as the membrane hydraulic conductivity. It is the purpose of this work to examine the osmotic response of bull sperm to sucrose and NaCl utilizing electron spin resonance (ESR) to measure cell volume. For calibration purposes we also measured the ESR response of human red cells (RBC), the osmotic response of which is well documented with other methods. 15 refs., 1 fig.

  2. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2–δAs2

    DOE PAGES

    Luo, Yongkang; Ronning, F.; Wakeham, N.; ...

    2015-10-19

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2–δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressuremore » and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 e–/formular unit in CeNi2–δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. Here, the small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening.« less

  3. Mode Analysis for Long-Term Behavior in a Resonant Earth-Moon Trajectory

    NASA Astrophysics Data System (ADS)

    Short, Cody; Howell, Kathleen; Haapala, Amanda; Dichmann, Donald

    2016-11-01

    Trajectory design in chaotic regimes allows for the exploitation of system dynamics to achieve certain behaviors. For example, for the Transiting Exoplanet Survey Satellite (TESS) mission, the selected science orbit represents a stable option well-suited to meet the mission objectives. Extended analysis of particular solutions nearby in the phase space reveals transitions into desirable terminal modes induced by natural dynamics. This investigation explores the trajectory behavior and borrows from flow-based analysis strategies to characterize modes of such a motion. Perturbed initial states from a TESS-like orbit are evolved to supply motion suitable for contingency analysis. Through the associated analysis, mechanisms are identified that drive the spacecraft into particular modes and supply conditions necessary for such transitions.

  4. Magnetic field and in situ stress dependence of elastic behavior in EuTiO3 from resonant ultrasound spectroscopy

    NASA Astrophysics Data System (ADS)

    Schiemer, Jason; Spalek, Leszek J.; Saxena, Siddharth S.; Panagopoulos, Christos; Katsufuji, Takuro; Bussmann-Holder, Annette; Köhler, Jürgen; Carpenter, Michael A.

    2016-02-01

    Magnetoelectric coupling phenomena in EuTiO3 are of considerable fundamental interest and are also understood to be key to reported multiferroic behavior in strained films, which exhibit distinctly different properties to the bulk. Here, the magnetoelastic coupling of EuTiO3 is investigated by resonant ultrasound spectroscopy with in situ applied magnetic field and stress as a function of temperature ranging from temperatures above the structural transition temperature T s to below the antiferromagnetic ordering temperature T n. One single crystal and two polycrystalline samples are investigated and compared to each other. Both paramagnetic and diamagnetic transducer carriers are used, allowing an examination of the effect of both stress and magnetic field on the behavior of the sample. The properties are reported in constant field/variable temperature and in constant temperature/variable field mode where substantial differences between both data sets are observed. In addition, elastic and magnetic poling at high fields and stresses at low temperature has been performed in order to trace the history dependence of the elastic constants. Four different temperature regions are identified, characterized by unusual elastic responses. The low-temperature phase diagram has been explored and found to exhibit rich complexity. The data evidence a considerable relaxation of elastic constants at high temperatures, but with little effect from magnetic field alone above 20 K, in addition to the known low-temperature coupling.

  5. Behavioral, blood, and magnetic resonance imaging biomarkers of experimental mild traumatic brain injury

    PubMed Central

    Wright, David K.; Trezise, Jack; Kamnaksh, Alaa; Bekdash, Ramsey; Johnston, Leigh A.; Ordidge, Roger; Semple, Bridgette D.; Gardner, Andrew J.; Stanwell, Peter; O’Brien, Terence J.; Agoston, Denes V.; Shultz, Sandy R.

    2016-01-01

    Repeated mild traumatic brain injuries (mTBI) may lead to serious neurological consequences, especially if re-injury occurs within the period of increased cerebral vulnerability (ICV) triggered by the initial insult. MRI and blood proteomics might provide objective measures of pathophysiological changes in mTBI, and indicate when the brain is no longer in a state of ICV. This study assessed behavioral, MRI, and blood-based markers in a rat model of mTBI. Rats were given a sham or mild fluid percussion injury (mFPI), and behavioral testing, MRI, and blood collections were conducted up to 30 days post-injury. There were cognitive impairments for three days post-mFPI, before normalizing by day 5 post-injury. In contrast, advanced MRI (i.e., tractography) and blood proteomics (i.e., vascular endothelial growth factor) detected a number of abnormalities, some of which were still present 30 days post-mFPI. These findings suggest that MRI and blood proteomics are sensitive measures of the molecular and subtle structural changes following mTBI. Of particular significance, this study identified novel tractography measures that are able to detect mTBI and may be more sensitive than traditional diffusion-tensor measures. Furthermore, the blood and MRI findings may have important implications in understanding ICV and are translatable to the clinical setting. PMID:27349514

  6. Numerical approach to time-dependent quantum transport and dynamical Kondo transition.

    PubMed

    Zheng, Xiao; Jin, Jinshuang; Welack, Sven; Luo, Meng; Yan, YiJing

    2009-04-28

    An accurate and efficient numerical approach is developed for the transient electronic dynamics of open quantum systems at low temperatures. The calculations are based on a formally exact hierarchical equations of motion quantum dissipation theory [J. S. Jin et al., J. Chem. Phys. 128, 234703 (2008)]. We propose a hybrid scheme that combines the Matsubara expansion technique and a frequency dispersion treatment to account for reservoir correlation functions. The new scheme not just admits various forms of reservoir spectral functions but also greatly reduces the computational cost of the resulting hierarchical equations, especially in the low temperature regime. Dynamical Kondo effects are obtained and the cotunneling induced Kondo transitions are resolved in the transient current in response to time-dependent external voltages.

  7. Superconductivity of composite particles in a two-channel Kondo lattice.

    PubMed

    Hoshino, Shintaro; Kuramoto, Yoshio

    2014-04-25

    Emergence of odd-frequency s-wave superconductivity is demonstrated in the two-channel Kondo lattice by means of the dynamical mean-field theory combined with the continuous-time quantum Monte Carlo method. Around half filling of the conduction bands, divergence of an odd-frequency pairing susceptibility is found, which signals instability toward the superconductivity. The corresponding order parameter is equivalent to a staggered composite-pair amplitude with even frequencies, which involves both localized spins and conduction electrons. A model wave function is constructed for the composite order with the use of symmetry operations such as charge conjugation and channel rotations. Given a certain asymmetry of the conduction bands, another s-wave superconductivity is found that has a uniform order parameter. The Kondo effect in the presence of two channels is essential for both types of unconventional superconductivity.

  8. Layered Kondo lattice model for quantum critical beta-YbAlB4.

    PubMed

    Nevidomskyy, Andriy H; Coleman, P

    2009-02-20

    We analyze the magnetic and electronic properties of the quantum critical heavy fermion superconductor beta-YbAlB4, calculating the Fermi surface and the angular dependence of the extremal orbits relevant to the de Haas-van Alphen measurements. Using a combination of the realistic materials modeling and single-ion crystal field analysis, we are led to propose a layered Kondo lattice model for this system, in which two-dimensional boron layers are Kondo coupled via interlayer Yb moments in a Jz=+/-5/2 state. This model fits the measured single-ion magnetic susceptibility and predicts a substantial change in the electronic anisotropy as the system is pressure tuned through the quantum critical point.

  9. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    PubMed Central

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; Gu, Genda; Mason, Nadya

    2016-01-01

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. We characterize the zero-bias peaks and discuss their origin. PMID:26911258

  10. Ionic Hamiltonians for transition metal atoms: effective exchange coupling and Kondo temperature

    NASA Astrophysics Data System (ADS)

    Flores, F.; Goldberg, E. C.

    2017-02-01

    An ionic Hamiltonian for describing the interaction between a metal and a d-shell transition metal atom having an orbital singlet state is introduced and its properties analyzed using the Schrieffer-Wolf transformation (exchange coupling) and the poor man’s scaling method (Kondo temperature). We find that the effective exchange coupling between the metal and the atom has an antiferromagnetic or a ferromagnetic interaction depending on the kind of atomic fluctuations, either S\\to S-1/2 or S\\to S+1/2 , associated with the metal-atom coupling. We present a general scheme for all those processes and calculate, for the antiferromagnetic interaction, the corresponding Kondo-temperature.

  11. Spiral magnetic phases on the Kondo Lattice Model: A Hartree-Fock approach

    NASA Astrophysics Data System (ADS)

    Costa, N. C.; Lima, J. P.; dos Santos, Raimundo R.

    2017-02-01

    We study the Kondo Lattice Model (KLM) on a square lattice through a Hartree-Fock approximation in which the local spins are treated semi-classically, in the sense that their average values are modulated by a magnetic wavevector Q while they couple with the conduction electrons through fermion operators. In this way, we obtain a ground state phase diagram in which spiral magnetic phases (in which the wavevector depends on the coupling constants and on the density) interpolate between the low-density ferromagnetic phase and the antiferromagnetic phase at half filling; within small regions of the phase diagram commensurate magnetic phases can coexist with Kondo screening. We have also obtained 'Doniach-like' diagrams, showing the effect of temperature on the ground state phases, and established that for some ranges of the model parameters (the exchange coupling and conduction electron density) the magnetic wavevector changes with temperature, either continuously or abruptly (e.g., from spiral to ferromagnetic).

  12. Excitons in topological Kondo insulators: Theory of thermodynamic and transport anomalies in SmB6

    NASA Astrophysics Data System (ADS)

    Knolle, Johannes; Cooper, Nigel R.

    2017-03-01

    Kondo insulating materials lie outside the usual dichotomy of weakly versus correlated—band versus Mott—insulators. They are metallic at high temperatures but resemble band insulators at low temperatures because of the opening of an interaction-induced band gap. The first discovered Kondo insulator (KI) SmB6 has been predicted to form a topological KI (TKI). However, since its discovery thermodynamic and transport anomalies have been observed that have defied a theoretical explanation. Enigmatic signatures of collective modes inside the charge gap are seen in specific heat, thermal transport, and quantum oscillation experiments in strong magnetic fields. Here, we show that TKIs are susceptible to the formation of excitons and magnetoexcitons. These charge neutral composite particles can account for long-standing anomalies in SmB6 .

  13. Jahn-Teller / Kondo Interplay in a Three-Terminal Quantum Dot

    NASA Astrophysics Data System (ADS)

    Toonen, R. C.; Qin, H.; Huettel, A. K.; Goswami, S.; van der Weide, D. W.; Eberl, K.; Blick, R. H.

    2006-03-01

    The Jahn-Teller effect is the spontaneous geometric distortion of a nonlinear molecular entity. The Kondo effect, an expression of asymptotic freedom, arises from the hybridization between localized states of a magnetic impurity and the itinerant states of its environment. The interplay of these two phenomena has attracted the attention of theorists studying the growth and interactions of heavy-fermion systems. Because of the technical difficulties associated with probing isolated impurities in bulk materials, this composite effect has remained experimentally unexplored. We have investigated co-tunneling transport phenomena in a three-terminal quantum dot with triangular symmetry. Our measurements of anomalous spectral signatures reveal interplay between the Jahn-Teller and Kondo effects. This discovery suggests a means of controlling the correlation of spatially separated pairs of entangled electrons (EPR pairs)---a necessary condition for the physical realization of a quantum computer (DiVincenzo's 7th requirement).

  14. Kondo lattice on the edge of a 2D topological insulator

    NASA Astrophysics Data System (ADS)

    Maciejko, Joseph

    2012-02-01

    Much attention has been devoted recently to the experimental and theoretical study of the effect of magnetic impurities on the stability of the gapless boundary modes of topological insulators. When the quantum dynamics of the impurities is considered, those boundary modes constitute novel types of fermionic baths which may affect the nature of possible impurity phases and phase transitions. We study a regular one-dimensional array of quantum magnetic impurities interacting with the helical edge liquid of a two-dimensional time-reversal invariant topological insulator. Exact solutions at the special Toulouse and Luther-Emery points as well as a renormalization group analysis àla Anderson-Yuval allow us to construct a phase diagram in the space of Kondo coupling, electron-electron interaction strength, and electron density. We point out similarities and differences with the Kondo lattice in a ordinary one-dimensional electron gas.

  15. Excitons in topological Kondo insulators: Theory of thermodynamic and transport anomalies in SmB_{6}.

    PubMed

    Knolle, Johannes; Cooper, Nigel R

    2017-03-03

    Kondo insulating materials lie outside the usual dichotomy of weakly versus correlated-band versus Mott-insulators. They are metallic at high temperatures but resemble band insulators at low temperatures because of the opening of an interaction-induced band gap. The first discovered Kondo insulator (KI) SmB_{6} has been predicted to form a topological KI (TKI). However, since its discovery thermodynamic and transport anomalies have been observed that have defied a theoretical explanation. Enigmatic signatures of collective modes inside the charge gap are seen in specific heat, thermal transport, and quantum oscillation experiments in strong magnetic fields. Here, we show that TKIs are susceptible to the formation of excitons and magnetoexcitons. These charge neutral composite particles can account for long-standing anomalies in SmB_{6}.

  16. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    SciTech Connect

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; Gu, Genda; Mason, Nadya

    2016-02-25

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. As a result, we characterize the zero-bias peaks and discuss their origin.

  17. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    DOE PAGES

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; ...

    2016-02-25

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. As a result, we characterize the zero-bias peaks and discuss their origin.

  18. Thermodynamic Investigation of Metamagnetic Transitions and Partial Disorder in the Quasi-Kagome Kondo Lattice CePdAl

    NASA Astrophysics Data System (ADS)

    Mochidzuki, Kenji; Shimizu, Yusei; Kondo, Akihiro; Nakamura, Shota; Kittaka, Shunichiro; Kono, Yohei; Sakakibara, Toshiro; Ikeda, Yoichi; Isikawa, Yosikazu; Kindo, Koichi

    2017-03-01

    Low-temperature (T) thermodynamic properties of the quasi-Kagome antiferromagnet CePdAl (TN ˜ 2.7 K) in magnetic fields (B) were studied by magnetization and specific-heat C(T, B) measurements. The unusual magnetic phase diagram, including three thermodynamic phases I-III and crossover anomalies, has been obtained. In the low-field phase I, the existence of the partial Kondo screening state on one-third of the Ce sites is supported from the following thermodynamic view points: (i) the appearance of a paramagnetic moment with one-third of the full moment around 3 T and (ii) the occurrence of an entropy release of ˜0.3R ln 2 around the observed crossover. On the other hand, a strong enhancement of C/T was found around the point where TN(B) meets the boundary of phase III, indicating the possible presence of a tricritical point. Furthermore, it is suggested that the three metamagnetic transitions at Bmi (i = 1,2,3) originate from successive increments of the Ising-type magnetic moment along the c-axis. In the high-field region above 20 T, the behavior of f electrons can be roughly described by the crystal-electric-field model.

  19. Strongly correlated electron physics: From Kondo and spin glasses to heavy fermions, hidden order and quantum phase transitions

    NASA Astrophysics Data System (ADS)

    Bennett, Edmund; Mydosh, J. A.

    2012-09-01

    We summarize the development of strongly correlated electron physics (SCEP) stimu-lated from the 1930's when a strange upturn was found in the electrical resistivity at low temper-atures. It was only in 1965 that this effect was explained as a many-body, spin-flip, scattering of electrons from a magnetic impurity, i.e., the Kondo effect. This marked the beginning of SCEP. When the concentration of these impurities is increased so that they can randomly interact we have the spin glasses and their unconventional, yet classical phase transition. Spin glass physics formed the background know-how for the combination of two ferromagnetic layers separated by a non-magnetic spacer which generated the the giant magnetic resistance and it many applications in com-puter hardware. By fabricating a lattice of the magnetic species, viz., an intermetallic compound based upon certain rare-earth and actinide elements, we then create a heavy Fermi liquid that can support most unusual ground-state behavior, e.g., unconventional superconductivity. This leads to the mysterious and still unexplained "hidden order" phase transition of URu2Si2. Finally, since the heavy fermions commonly exhibit zero temperature phase transitions, aka, quantum phase transitions when tuned with pressure, magnetic field or doping, we are at the summit of today's SCEP - the prime topic of 2012 condensed matter physics.

  20. Phase diagram of the Kondo lattice model with a superlattice potential

    NASA Astrophysics Data System (ADS)

    Silva-Valencia, J.; Franco, R.; Figueira, M. S.

    2016-02-01

    We study the ground state of a Kondo lattice model where the free carries undergo a superlattice potential. Using the density matrix renormalization group method, we establish that the model exhibits a ferromagnetic phase and spiral phase whose boundaries in the phase diagram depend on the depth of the potential. Also, we observed that the spiral to ferromagnetic quantum phase transition can be tuned by changing the local coupling or the superlattice strength.

  1. Transport properties of a multichannel Kondo dot in a magnetic field

    NASA Astrophysics Data System (ADS)

    Hörig, Christoph B. M.; Schuricht, Dirk

    2012-04-01

    We study the nonequilibrium transport through a multichannel Kondo quantum dot in the presence of a magnetic field. We use the exact solution of the two-loop renormalization group equation to derive analytical results for the g factor, the spin relaxation rates, the magnetization, and the differential conductance. We show that the finite magnetization leads to a coupling between the conduction channels, which manifests itself in additional features in the differential conductance.

  2. Kondo spin screening cloud in two-dimensional electron gas with spin-orbit couplings.

    PubMed

    Feng, Xiao-Yong; Zhang, Fu-Chun

    2011-03-16

    A spin-1/2 Anderson impurity in a semiconductor quantum well with Rashba and Dresselhaus spin-orbit couplings is studied by using a variational wavefunction method. The local magnetic moment is found to be quenched at low temperatures. The spin-spin correlations of the impurity and the conduction electron density show anisotropy in both spatial and spin spaces, which interpolates the Kondo spin screenings of a conventional metal and of a surface of three-dimensional topological insulators.

  3. Transport in a hybrid normal metal/topological superconductor Kondo model

    NASA Astrophysics Data System (ADS)

    Chirla, Razvan; Dinu, I. V.; Moldoveanu, V.; Moca, Cǎtǎlin Paşcu

    2014-11-01

    We investigate the equilibrium and nonequilibrium transport through a quantum dot in the Kondo regime, embedded between a normal metal and a topological superconductor supporting Majorana bound states at its end points. We find that the Kondo physics is significantly modified by the presence of the Majorana modes. When the Majorana modes are coupled, aside from the Kondo scale TK, a new energy scale T*≪TK emerges, that controls the low-energy physics of the system. At low temperatures, the ac conductance is suppressed for frequencies below T*, while the noise spectrum acquires a ˜ω3 dependence. At high temperatures, T ≫TK , the regular logarithmic dependence in the differential conductance is also affected. Under nonequilibrium conditions, and in particular in the {T ,B }→0 limit, the differential conductance becomes negative. These findings indicate that the changes in transport may serve as clues for detecting the Majorana bound states in such systems. In terms of methods used, we characterize the transport by using a combination of perturbative and renormalization-group approaches.

  4. Controlling Kondo-like Scattering at the SrTiO3-based Interfaces

    PubMed Central

    Han, K.; Palina, N.; Zeng, S. W.; Huang, Z.; Li, C. J.; Zhou, W. X.; Wan, D.-Y.; Zhang, L. C.; Chi, X.; Guo, R.; Chen, J. S.; Venkatesan, T.; Rusydi, A.; Ariando, A

    2016-01-01

    The observation of magnetic interaction at the interface between nonmagnetic oxides has attracted much attention in recent years. In this report, we show that the Kondo-like scattering at the SrTiO3-based conducting interface is enhanced by increasing the lattice mismatch and growth oxygen pressure PO2. For the 26-unit-cell LaAlO3/SrTiO3 (LAO/STO) interface with lattice mismatch being 3.0%, the Kondo-like scattering is observed when PO2 is beyond 1 mTorr. By contrast, when the lattice mismatch is reduced to 1.0% at the (La0.3Sr0.7)(Al0.65Ta0.35)O3/SrTiO3 (LSAT/STO) interface, the metallic state is always preserved up to PO2 of 100 mTorr. The data from Hall measurement and X-ray absorption near edge structure (XANES) spectroscopy reveal that the larger amount of localized Ti3+ ions are formed at the LAO/STO interface compared to LSAT/STO. Those localized Ti3+ ions with unpaired electrons can be spin-polarized to scatter mobile electrons, responsible for the Kondo-like scattering observed at the LAO/STO interface. PMID:27147407

  5. Understanding Quantum Transport and the Kondo Effect in 2D Carbon Systems

    NASA Astrophysics Data System (ADS)

    McIntosh, Ross; Churochkin, Dmitry; Bhattacharyya, Somnath

    2013-03-01

    The rich physics surrounding correlations between conduction electrons and local spins in quantum dot systems is of significant interest towards the development of spintronic quantum information devices. In this study we establish the Kondo effect in reduced graphene oxide (RGO) films through a metal-insulator transition in resistance versus temperature interpreted within the Fermi liquid description of the Kondo effect and negative magnetoresistance which scales with a Kondo characteristic temperature. With a microstructure consisting of intact graphene nano-islands embedded within residual functionalized regions where local magnetic moments may form, RGO is effectively a disordered quantum dot system. This work is augmented with a theoretical study of transport through nano-scale multiple quantum dot devices. Solving within a Keldysh formalism we scrutinize quasi-bound state formation in a range of geometrical quantum dot configurations in order to interpret coherent quantum interference effects. We demonstrate negative differential conductance and control over device parameters such as the characteristic time. This tandem approach illustrates the promise of innovative low dimensional carbon spintronic devices.

  6. Kondo screening of Andreev bound states in a normal metal-quantum dot-superconductor system

    NASA Astrophysics Data System (ADS)

    Li, Lin; Cao, Zhan; Fang, Tie-Feng; Luo, Hong-Gang; Chen, Wei-Qiang

    2016-10-01

    Motivated by experimental observation of the Kondo-enhanced Andreev transport [R. S. Deacon et al., Phys. Rev. B 81, 121308(R) (2010), 10.1103/PhysRevB.81.121308] in a hybrid normal metal-quantum dot-superconductor (N-QD-S) device, we theoretically study the Kondo effect in such a device and clarify the different roles played by the normal and superconducting leads. Due to the Andreev reflection in a QD-S system, a pair of Andreev energy levels form in the superconducting gap, which is able to carry the magnetic moment if the ground state of the QD is a magnetic doublet. In this sense, the Andreev energy levels play a role of effective impurity levels. When the normal lead is coupled to the QD-S system, on the one hand, the Andreev energy levels broaden to form the so-called Andreev bound states (ABSs); on the other hand, it can screen the magnetic moment of the ABSs. By tuning the couplings between the QD and the normal (superconducting) leads, the ABSs can simulate the Kondo, mixed-valence, and even empty orbit regimes of the usual single-impurity Anderson model. The above picture is confirmed by the Green's function calculation of the hybrid N-QD-S Anderson model and is also able to explain qualitatively experimental phenomena observed by Deacon et al. These results can further stimulate related experimental study in the N-QD-S systems.

  7. Quantum phase transitions in the Kondo-necklace model: perturbative continuous unitary transformation approach.

    PubMed

    Hemmatiyan, S; Rahimi Movassagh, M; Ghassemi, N; Kargarian, M; Rezakhani, A T; Langari, A

    2015-04-22

    The Kondo-necklace model can describe magnetic low-energy limit of strongly correlated heavy fermion materials. There exist multiple energy scales in this model corresponding to each phase of the system. Here, we study quantum phase transition between the Kondo-singlet phase and the antiferromagnetic long-range ordered phase, and show the effect of anisotropies in terms of quantum information properties and vanishing energy gap. We employ the 'perturbative continuous unitary transformations' approach to calculate the energy gap and spin-spin correlations for the model in the thermodynamic limit of one, two, and three spatial dimensions as well as for spin ladders. In particular, we show that the method, although being perturbative, can predict the expected quantum critical point, where the gap of low-energy spectrum vanishes, which is in good agreement with results of other numerical and Green's function analyses. In addition, we employ concurrence, a bipartite entanglement measure, to study the criticality of the model. Absence of singularities in the derivative of concurrence in two and three dimensions in the Kondo-necklace model shows that this model features multipartite entanglement. We also discuss crossover from the one-dimensional to the two-dimensional model via the ladder structure.

  8. Incoherence-coherence crossover and low-temperature Fermi-liquid-like behavior in AFe2As2 (A  =  K, Rb, Cs): evidence from electrical transport properties

    NASA Astrophysics Data System (ADS)

    Xiang, Z. J.; Wang, N. Z.; Wang, A. F.; Zhao, D.; Sun, Z. L.; Luo, X. G.; Wu, T.; Chen, X. H.

    2016-10-01

    We study the normal-state transport properties of AFe2As2 (A  =  K, Rb and Cs) single crystals using Hall coefficient, resistivity and magnetoresistance (MR) measurements. In all three materials, the Hall coefficient R H shows a strong temperature dependence, which is typical for multi-band systems. In particular, R H develops an upturn below a characteristic temperature {{T}\\ast} , which is in agreement with the incoherence-coherence crossover reported in recent nuclear magnetic resonance studies. A Fermi-liquid-like state, characterized by T 2 behavior of the resistivity and a positive orbital MR obeying Kohler’s rule, emerges below T FL  ˜0.4 ~{{T}\\ast} . The superconducting transition temperature T c experiences a simultaneous suppression with {{T}\\ast} and T FL as the alkali ion’s radius increases from A  =  K to A  =  Cs, suggesting that the unconventional superconductivity in the AFe2As2 series is related to the strength of the electronic coherence. A phase diagram, similar to that in the heavy fermion Kondo lattice system, is obtained. Based on all the experimental evidence, we argue that the physical properties of this family of heavily hole-doped Fe-based superconductors are controlled by the hybridization between itinerant carriers and localized orbitals, and the Kondo scenario could be effective in such a case.

  9. Surface Plasmon Resonance Fiber Sensor for Real-Time and Label-Free Monitoring of Cellular Behavior

    PubMed Central

    Shevchenko, Yanina; Camci-Unal, Gulden; Cuttica, Davide F.; Dokmeci, Mehmet R.; Albert, Jacques; Khademhosseini, Ali

    2014-01-01

    This paper reports on the application of an optical fiber biosensor for real-time analysis of cellular behavior. Our findings illustrate that a fiber sensor manufactured from a traditional telecommunication fiber can be integrated into conventional cell culture equipment and used for real-time and label-free monitoring of cellular responses to chemical stimuli. The sensing mechanism used for the measurement of cellular responses is based on the excitation of Surface Plasmon Resonance (SPR) on the surface of the optical fiber. In this proof of concept study, the sensor was utilized to investigate the influence of a number of different stimuli on cells - we tested the effects of trypsin, serum and sodium azide. These stimuli induced detachment of cells from the sensor surface, uptake of serum and inhibition of cellular metabolism, accordingly. The effects of different stimuli were confirmed with alamar blue assay, phase contrast and fluorescence microscopy. The results indicated that the fiber biosensor can be successfully utilized for real-time and label-free monitoring of cellular response in the first 30 minutes following the introduction of a stimulus. Furthermore, we demonstrated that the optical fiber biosensors can be easily regenerated for repeated use, proving this platform as a versatile and cost-effective sensing tool. PMID:24549115

  10. Orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films

    SciTech Connect

    Zhu, L. J.; Nie, S. H.; Xiong, P.; Schlottmann, P.; Zhao, J. H.

    2016-02-24

    The orbital two-channel Kondo effect displaying exotic non-Fermi liquid behaviour arises in the intricate scenario of two conduction electrons compensating a pseudo-spin-1/2 impurity of two-level system. Despite extensive efforts for several decades, no material system has been clearly identified to exhibit all three transport regimes characteristic of the two-channel Kondo effect in the same sample, leaving the interpretation of the experimental results a subject of debate. Here we present a transport study suggestive of a robust orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films, as evidenced by a magnetic field-independent resistivity upturn with a clear transition from logarithmic- to square-root temperature dependence and deviation from it in three distinct temperature regimes. Lastly, our results also provide an experimental indication of the presence of two-channel Kondo physics in a ferromagnet, pointing to considerable robustness of the orbital two-channel Kondo effect even in the presence of spin polarization of the conduction electrons.

  11. Field-Enhanced Kondo Correlations in a Half-Filling Nanotube Dot: Evolution of an SU(N) Fermi-Liquid Fixed Point

    NASA Astrophysics Data System (ADS)

    Teratani, Yoshimichi; Sakano, Rui; Fujiwara, Ryo; Hata, Tokuro; Arakawa, Tomonori; Ferrier, Meydi; Kobayashi, Kensuke; Oguri, Akira

    2016-09-01

    Carbon nanotube quantum dot has four-fold degenerate one-particle levels, which bring a variety to the Kondo effects taking place in a wide tunable-parameter space. We theoretically study an emergent SU(2) symmetry that is suggested by recent magneto-transport measurements, carried out near two electrons filling. It does not couple with the magnetic field, and emerges in the case where the spin and orbital Zeeman splittings cancel each other out in two of the one-particle levels among four. This situation seems to be realized in the recent experiment. Using the Wilson numerical renormalization group, we show that a crossover from the SU(4) to SU(2) Fermi-liquid behavior occurs as magnetic field increases at two impurity-electrons filling. We also find that the quasiparticles are significantly renormalized as the remaining two one-particle levels move away from the Fermi level and are frozen at high magnetic fields. Furthermore, we consider how the singlet ground state evolves during such a crossover. Specifically, we reexamine the SU(N) Kondo singlet for M impurity-electrons filling in the limit of strong exchange interactions. We find that the nondegenerate Fermi-liquid fixed point of Nozières and Blandin can be described as abosonic Perron-Frobenius vector for M composite pairs, each of which consists of one impurity-electron and one conduction-hole. This interpretation in terms of the Perron-Frobenius theorem can also be extended to the Fermi-liquid fixed-point without the SU(N) symmetry.

  12. Kondo Impurities in the Kitaev Spin Liquid: Numerical Renormalization Group Solution and Gauge-Flux-Driven Screening.

    PubMed

    Vojta, Matthias; Mitchell, Andrew K; Zschocke, Fabian

    2016-07-15

    Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.

  13. The Ising-Anisotropic Kondo Lattice in a transverse field: EDMFT study and implications for the global phase diagram

    NASA Astrophysics Data System (ADS)

    Nica, Emilian Marius; Ingersent, Kevin; Si, Qimiao

    2015-03-01

    Heavy-fermion materials exhibit a rich variety of phase transitions. Of particular interest are quantum phase transitions and the associated breakdown of the Fermi liquid picture. A theoretical example of this is the Kondo destruction effect in the context of local quantum criticality. To capture this effect and others, a zero-temperature global phase diagram for heavy-fermion materials has been proposed. It incorporates the competition between the Kondo effect (promoted by exchange coupling JK) and the variable quantum fluctuations of the local-moment magnetism (parameterized by G). We investigate this competition in the Ising-anisotropic Kondo lattice with a transverse magnetic field, where the field serves to tune G. We determine a zero-temperature phase diagram of this model within the extended dynamical mean-field theory (EDMFT), and discuss the implications of our results for the global phase diagram of heavy-fermion systems.

  14. Microscopic resolution of the interplay of Kondo screening and superconducting pairing: Mn-phthalocyanine molecules adsorbed on superconducting Pb(111)

    NASA Astrophysics Data System (ADS)

    Bauer, Johannes; Pascual, Jose I.; Franke, Katharina J.

    2013-02-01

    Magnetic molecules adsorbed on a superconductor give rise to a local competition of Cooper pair and Kondo singlet formation inducing subgap bound states. For manganese-phthalocyanine molecules on a Pb(111) substrate, scanning tunneling spectroscopy resolves pairs of subgap bound states and two Kondo screening channels. We show in a combined approach of scaling and numerical renormalization group calculations that the intriguing relation between Kondo screening and superconducting pairing is solely determined by the hybridization strength with the substrate. We demonstrate that an effective one-channel Anderson impurity model with a sizable particle-hole asymmetry captures universal and nonuniversal observations in the system quantitatively. The model parameters and disentanglement of the two screening channels are elucidated by scaling arguments.

  15. Out-of-equilibrium Kondo effect in a quantum dot: Interplay of magnetic field and spin accumulation

    NASA Astrophysics Data System (ADS)

    Sahoo, Shaon; Crépieux, Adeline; Lavagna, Mireille

    2016-12-01

    We present a theoretical study of low-temperature nonequilibrium transport through an interacting quantum dot in the presence of Zeeman magnetic field and current injection into one of its leads. By using a self-consistent renormalized equation of motion approach, we show that the injection of a spin-polarized current leads to a modulation of the Zeeman splitting of the Kondo peak in the differential conductance. We find that an appropriate amount of spin accumulation in the lead can restore the Kondo peak by compensating the splitting due to magnetic field. By contrast when the injected current is spin-unpolarized, we establish that both Zeeman-split Kondo peaks are equally shifted and the splitting remains unchanged. Our results quantitatively explain the experimental findings reported in Kobayashi T. et al., Phys. Rev. Lett., 104 (2010) 036804. These features could be nicely exploited for the control and manipulation of spin in nanoelectronic and spintronic devices.

  16. Non-Kondo-like electronic structure in the correlated rare-earth hexaboride YbB(6).

    PubMed

    Neupane, Madhab; Xu, Su-Yang; Alidoust, Nasser; Bian, Guang; Kim, D J; Liu, Chang; Belopolski, I; Chang, T-R; Jeng, H-T; Durakiewicz, T; Lin, H; Bansil, A; Fisk, Z; Hasan, M Z

    2015-01-09

    We present angle-resolved photoemission studies on the rare-earth-hexaboride YbB(6), which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB(6) exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB(6) has three 2D Dirac cone like surface states enclosing the Kramers's points, while the f orbital that would be relevant for the Kondo mechanism is ∼1  eV below the Fermi level. Our first-principles calculation shows that the topological state that we observe in YbB(6) is due to an inversion between Yb d and B p bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.

  17. The advantage of linear viscoelastic material behavior in passive damper design-with application in broad-banded resonance dampers for industrial high-precision motion stages

    NASA Astrophysics Data System (ADS)

    Verbaan, Cornelis A. M.; Peters, Gerrit W. M.; Steinbuch, Maarten

    2017-01-01

    In this paper we demonstrate the advantage of applying viscoelastic materials instead of purely viscous materials as damping medium in mechanical dampers. Although the loss modulus decreases as function of frequency in case of viscoelastic behavior, which can be interpreted as a decrease of damping, the viscoelastic behavior still leads to an increased modal damping for mechanical structures. This advantage holds for inertial-mass-type dampers that are tuned for broad-banded resonance damping. It turns out that an increase of the storage modulus as function of frequency contributes to the effectiveness of mechanical dampers with respect to energy dissipation at different mechanical resonance frequencies. It is shown that this phenomenon is medium specific and is independent of the amount of damper mass.

  18. Effect of the repulsion interaction on the ground-state of the Kondo lattice model with a superlattice potential

    NASA Astrophysics Data System (ADS)

    Silva-Valencia, J.; Franco, R.; Figueira, M. S.

    2014-04-01

    We investigate the ground-state of a new Kondo lattice model, where the free carriers interact repulsively between them and undergo an external superlattice potential. This model can be simulated with 171Yb atoms confined in optical lattices. We use the density matrix renormalization group method to evaluate the charge and spin gaps, and the structure factors. We found that the ground-state evolves from a Kondo spin liquid state to a charge-gapped antiferromagnetic state with zero spin gap, when the antiferromagnetic exchange increases. Also, we verify that the quantum critical point varies linearly with the repulsion and the exchange.

  19. Development of a phantom mimicking the functional and structural behaviors of the thigh muscles characterized with magnetic resonance elastography technique.

    PubMed

    Chakouch, Mashhour K; Charleux, Fabrice; Bensamoun, Sabine F

    2015-01-01

    Magnetic Resonance Elastography (MRE) is a non invasive technique based on the propagation of shear waves in soft tissues providing the quantification of the mechanical properties [1]. MRE was successfully applied to healthy and pathological muscles. However, the MRE muscle methods must be further improved to characterize the deep muscles. A way will be to develop phantom mimicking the muscle behavior in order to set up new MRE protocol. Thus, the purpose of this study is to create a phantom composed of a similar skeletal muscle architecture (fiber, aponorosis) and equivalent elastic properties as a function of the muscle state (passive or active). Two homogeneous phantoms were manufactured with different concentrations of plastisol to simulate the elastic properties in relaxed (50% of plastisol) and contracted (70% of plastisol) muscle conditions. Moreover, teflon tubing pipes (D = 0.9 mm) were thread in the upper part of the phantom (50%) to represent the muscle fibers and a plastic sheet (8 × 15 cm) was also included in the middle of the phantom to mimic the aponeurosis structure. Subsequently, MRE tests were performed with two different pneumatic drivers, tube and round, (f = 90Hz) to analyze the effect of the type of driver on the wave propagation. Then, the wavelength was measured from the phase images to obtain the elastic properties (shear modulus). Both phantoms revealed elastic properties which were in the same range as in vivo muscle in passive (μ(50%) = 2.40 ± 0.18 kPa ) and active (6.24 ± 0.21 kPa) states. The impact of the type of driver showed higher values (about 1.2kPa) with the tube. The analysis of the wave behavior revealed a sliding along the plastic sheet as it was observed for in vivo muscle study. The wave was also sensitive to the presence of the fibers where gaps were identified. The present study demonstrates the ability of the phantom to mimic the structural and functional properties of the muscle.

  20. Limit Cycle and Anomalous Capacitance in the Kondo Insulator SmB6

    NASA Astrophysics Data System (ADS)

    Kim, D. J.; Grant, T.; Fisk, Z.

    2012-08-01

    We report a frequency coding limit cycle and anomalous capacitance in the Kondo insulator SmB6 at low temperatures where the insulating gap becomes fully opened. The limit cycle appears to be associated with local activity and autocatalytic temporal pattern formation, as occurs in biological systems. The measured anomalous capacitance may indicate surface and bulk separation, suggesting the formation of a surface conducting state. The biological analogy suggests lossless information transport and complex information coding, and the surface state with a superconductor would provide a possible venue for quantum computing resources without decoherence.

  1. Competition between Kondo Screening and Indirect Magnetic Exchange in a Quantum Box

    NASA Astrophysics Data System (ADS)

    Schwabe, Andrej; Gütersloh, Daniel; Potthoff, Michael

    2012-12-01

    Nanoscale systems of metal atoms antiferromagnetically exchange coupled to several magnetic impurities are shown to exhibit an unconventional reentrant competition between Kondo screening and indirect magnetic exchange interaction. Depending on the atomic positions of the magnetic moments, the total ground-state spin deviates from predictions of standard Ruderman-Kittel-Kasuya-Yosida perturbation theory. The effect shows up on an energy scale larger than the level width induced by the coupling to the environment and is experimentally accessible by studying magnetic field dependencies.

  2. Magnetically tunable Kondo-Aharonov-Bohm effect in a triangular quantum dot.

    PubMed

    Kuzmenko, T; Kikoin, K; Avishai, Y

    2006-02-03

    The role of discrete orbital symmetry in mesoscopic physics is manifested in a system consisting of three identical quantum dots forming an equilateral triangle. Under a perpendicular magnetic field, this system demonstrates a unique combination of Kondo and Aharonov-Bohm features due to an interplay between continuous [spin-rotation SU(2)] and discrete (permutation C3v) symmetries, as well as U(1) gauge invariance. The conductance as a function of magnetic flux displays sharp enhancement or complete suppression depending on contact setups.

  3. Vibration-induced Kondo tunneling through metal-organic complexes with even electron occupation number.

    PubMed

    Kikoin, K; Kiselev, M N; Wegewijs, M R

    2006-05-05

    We investigate transport through a mononuclear transition-metal complex with strong tunnel coupling to two electrodes. The ground state of this molecule is a singlet, while the first excited state is a triplet. We show that a modulation of the tunnel-barrier due to a molecular distortion which couples to the tunneling induces a Kondo-effect, provided the discrete vibrational energy compensates the singlet-triplet gap. We discuss the single-phonon and two-phonon-assisted cotunneling and possible experimental realization of the theory.

  4. Two-channel Kondo effect and the low-temperature crossover

    NASA Astrophysics Data System (ADS)

    Keller, Andrew; Peeters, Lucas; Weymann, Ireneusz; Moca, Cătălin Paşcu; Mahalu, Diana; Umansky, Vladimir; Zaránd, Gergely; Goldhaber-Gordon, David

    2015-03-01

    The two-channel Kondo (2CK) state, where a spin-1/2 impurity is equally exchange-coupled to two independent reservoirs, is a canonical non-Fermi liquid state. Experimental observations are rare because of its sensitivity to common and hard-to-control perturbations. We implement experimentally a 2CK state in a coupled dot-grain system (Potok, et al., doi:10.1038/nature05556), and explore the physics of the low-temperature crossover: how magnetic field and gate voltage drive the system towards a Fermi liquid ground state. Our experimental findings are corroborated by detailed numerical renormalization group modeling of our device.

  5. Long range order and two-fluid behavior in heavy electron materials

    DOE PAGES

    Shirer, Kent R.; Shockley, Abigail C.; Dioguardi, Adam P.; ...

    2012-09-24

    The heavy electron Kondo liquid is an emergent state of condensed matter that displays universal behavior independent of material details. Properties of the heavy electron liquid are best probed by NMR Knight shift measurements, which provide a direct measure of the behavior of the heavy electron liquid that emerges below the Kondo lattice coherence temperature as the lattice of local moments hybridizes with the background conduction electrons. Because the transfer of spectral weight between the localized and itinerant electronic degrees of freedom is gradual, the Kondo liquid typically coexists with the local moment component until the material orders at lowmore » temperatures. The two-fluid formula captures this behavior in a broad range of materials in the paramagnetic state. In order to investigate two-fluid behavior and the onset and physical origin of different long range ordered ground states in heavy electron materials, we have extended Knight shift measurements to URu2Si2, CeIrIn5, and CeRhIn5. In CeRhIn5 we find that the antiferromagnetic order is preceded by a relocalization of the Kondo liquid, providing independent evidence for a local moment origin of antiferromagnetism. In URu2Si2 the hidden order is shown to emerge directly from the Kondo liquid and so is not associated with local moment physics. Lastly, our results imply that the nature of the ground state is strongly coupled with the hybridization in the Kondo lattice in agreement with phase diagram proposed by Yang and Pines.« less

  6. Long range order and two-fluid behavior in heavy electron materials

    SciTech Connect

    Shirer, Kent R.; Shockley, Abigail C.; Dioguardi, Adam P.; Crocker, John; Lin, Ching H.; apRoberts-Warren, Nicholas; Nisson, David M.; Klavins, Peter; Cooley, Jason C.; Yang, Yi -feng; Curro, Nicholas J.

    2012-09-24

    The heavy electron Kondo liquid is an emergent state of condensed matter that displays universal behavior independent of material details. Properties of the heavy electron liquid are best probed by NMR Knight shift measurements, which provide a direct measure of the behavior of the heavy electron liquid that emerges below the Kondo lattice coherence temperature as the lattice of local moments hybridizes with the background conduction electrons. Because the transfer of spectral weight between the localized and itinerant electronic degrees of freedom is gradual, the Kondo liquid typically coexists with the local moment component until the material orders at low temperatures. The two-fluid formula captures this behavior in a broad range of materials in the paramagnetic state. In order to investigate two-fluid behavior and the onset and physical origin of different long range ordered ground states in heavy electron materials, we have extended Knight shift measurements to URu2Si2, CeIrIn5, and CeRhIn5. In CeRhIn5 we find that the antiferromagnetic order is preceded by a relocalization of the Kondo liquid, providing independent evidence for a local moment origin of antiferromagnetism. In URu2Si2 the hidden order is shown to emerge directly from the Kondo liquid and so is not associated with local moment physics. Lastly, our results imply that the nature of the ground state is strongly coupled with the hybridization in the Kondo lattice in agreement with phase diagram proposed by Yang and Pines.

  7. PRESS echo time behavior of triglyceride resonances at 1.5 T: Detecting ω-3 fatty acids in adipose tissue in vivo

    NASA Astrophysics Data System (ADS)

    Lundbom, Jesper; Heikkinen, Sami; Fielding, Barbara; Hakkarainen, Antti; Taskinen, Marja-Riitta; Lundbom, Nina

    2009-11-01

    AimThis study investigated the impact of fatty acid (FA) composition on the echo time behavior of triglyceride resonances in a clinical setting. The feasibility of 1H NMR spectroscopy to detect these resonances was also evaluated in human adipose tissue in vivo. MethodTen edible oils chosen to cover a wide spectrum of FA compositions were used as phantom material. The detailed FA composition and intrinsic proton spectra of the oils were characterized by gas chromatography and high-resolution 1H NMR spectroscopy (11.7 T), respectively. The detailed echo time behavior of the oils were subsequently measured by 1H NMR spectroscopy in a clinical scanner (1.5 T) using PRESS. The effect of temperature was investigated in five oils. ResultsThe olefinic (5.3 ppm) and diallylic (2.8 ppm) resonances exhibited distinct J-modulation patterns independent of oil FA composition. The methylene resonance (1.3 ppm) displayed an exponential decay, with the apparent T2 showing a weak positive correlation with oil unsaturation ( R = 0.628, P = 0.052), probably a result of changes in viscosity. For the methyl resonance (0.9 ppm), oils high in ω-3 FA displayed a markedly different J-modulation pattern compared to non-ω-3 oils. The characteristic J-modulation of the ω-3 methyl group could be attributed to the phase behavior of the ω-3 methyl triplet signal (all triplet lines in-phase at TE of 135 ms), a result of the ω-3 methyl end forming a first order spin system. The ω-3 methyl outer triplet line at 1.08 ppm of the TE = 140 ms spectrum was found to be useful for determining the ω-3 content of the oils ( R = 0.999, standard error of estimate (SE) 0.80). The olefinic and diallylic proton resonance (measured at TE = 50 ms) areas correlated with the olefinic ( R = 0.993, SE 0.33) and diallylic ( R = 0.997, SE 0.19) proton contents calculated from the GC data. Information derived from long echo time spectra (TE = 200) demonstrated good correlations to GC data and showed no change with

  8. Magnetic order and Kondo effect in the Anderson-lattice model

    NASA Astrophysics Data System (ADS)

    Bernhard, B. H.; Aguiar, C.; Kogoutiouk, I.; Coqblin, B.

    The Anderson-lattice model has been extensively developed to account for the properties of many anomalous rare-earth compounds and in particular for the competition between the Kondo effect and an antiferromagnetic (AF) phase in a cubic lattice. Here we apply the higher-order decoupling of the equations of motion for the Green Functions (GF) introduced in [H.G. Luo, S.J. Wang, Phys. Rev. B 62 (2000) 1485]. We obtain an improved description of the phase diagram, where the AF phase subsists in a smaller range of the model parameters. As higher-order GF are included in the chain of equations, we are able to calculate directly the local spin-flip correlation function . As a further improvement to the previous approximation of [B.H. Bernhard, C. Aguiar, B. Coqblin, Physica B 378-380 (2006) 712], we obtain a reduced range of existence for the AF phase for the symmetric half-filled case and then we discuss the competition between the AF order and the Kondo effect as a function of the band filling.

  9. Possible undercompensation effect in the Kondo insulator (Yb,Tm)B12

    NASA Astrophysics Data System (ADS)

    Alekseev, P. A.; Nemkovski, K. S.; Mignot, J.-M.; Clementyev, E. S.; Ivanov, A. S.; Rols, S.; Bewley, R. I.; Filipov, V. B.; Shitsevalova, N. Yu.

    2014-03-01

    The effects of Tm substitution on the dynamical magnetic response of Yb1-xTmxB12 (x=0, 0.08, 0.15, and 0.75) and Lu0.92Tm0.08B12 compounds have been studied using time-of-flight inelastic neutron scattering. Major changes were observed in the spectral structure and temperature evolution of the Yb contribution to the inelastic response for a rather low content of magnetic Tm ions. A sizable influence of the RB12 host (YbB12, as compared to LuB12 or pure TmB12) on the crystal-field splitting of the Tm3+ ion is also reported. The results point to a specific effect of impurities carrying a magnetic moment (Tm, as compared to Lu or Zr) in a Kondo insulator, which is thought to reflect the "undercompensation" of Yb magnetic moments, originally Kondo screened in pure YbB12. A parallel is made with the strong effect of Tm substitution on the temperature dependence of the Seebeck coefficient in Yb1-xTmxB12, which was reported previously.

  10. Kondo effect in a neutral and stable all organic radical single molecule break junction

    NASA Astrophysics Data System (ADS)

    Burzuri, Enrique; Gaudenzi, Rocco; Frisenda, Riccardo; Franco, Carlos; Mas-Torrent, Marta; Rovira, Concepcio; Veciana, Jaume; Alcon, Isaac; Bromley, Stefan T.; van der Zant, Herre S. J.

    Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin-orbit coupling makes organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. We show that the paramagnetism of the PTM radical molecule, in the shape of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical specie. We further study polyradical systems, where several unpaired spins interact in the same molecule. This work was supported by the EU FP7 program through project 618082 ACMOL and ERC grant advanced Mols@Mols. It was also supported by the Dutch funding organization NWO (VENI).

  11. Formation of metallic magnetic clusters in a Kondo-lattice metal: evidence from an optical study.

    PubMed

    Kovaleva, N N; Kugel, K I; Bazhenov, A V; Fursova, T N; Löser, W; Xu, Y; Behr, G; Kusmartsev, F V

    2012-01-01

    Magnetic materials are usually divided into two classes: those with localised magnetic moments, and those with itinerant charge carriers. We present a comprehensive experimental (spectroscopic ellipsomerty) and theoretical study to demonstrate that these two types of magnetism do not only coexist but complement each other in the Kondo-lattice metal, Tb(2)PdSi(3). In this material the itinerant charge carriers interact with large localised magnetic moments of Tb(4f) states, forming complex magnetic lattices at low temperatures, which we associate with self-organisation of magnetic clusters. The formation of magnetic clusters results in low-energy optical spectral weight shifts, which correspond to opening of the pseudogap in the conduction band of the itinerant charge carriers and development of the low- and high-spin intersite electronic transitions. This phenomenon, driven by self-trapping of electrons by magnetic fluctuations, could be common in correlated metals, including besides Kondo-lattice metals, Fe-based and cuprate superconductors.

  12. Formation of metallic magnetic clusters in a Kondo-lattice metal: Evidence from an optical study

    NASA Astrophysics Data System (ADS)

    Kovaleva, N. N.; Kugel, K. I.; Bazhenov, A. V.; Fursova, T. N.; Löser, W.; Xu, Y.; Behr, G.; Kusmartsev, F. V.

    2012-11-01

    Magnetic materials are usually divided into two classes: those with localised magnetic moments, and those with itinerant charge carriers. We present a comprehensive experimental (spectroscopic ellipsomerty) and theoretical study to demonstrate that these two types of magnetism do not only coexist but complement each other in the Kondo-lattice metal, Tb2PdSi3. In this material the itinerant charge carriers interact with large localised magnetic moments of Tb(4f) states, forming complex magnetic lattices at low temperatures, which we associate with self-organisation of magnetic clusters. The formation of magnetic clusters results in low-energy optical spectral weight shifts, which correspond to opening of the pseudogap in the conduction band of the itinerant charge carriers and development of the low- and high-spin intersite electronic transitions. This phenomenon, driven by self-trapping of electrons by magnetic fluctuations, could be common in correlated metals, including besides Kondo-lattice metals, Fe-based and cuprate superconductors.

  13. Formation of metallic magnetic clusters in a Kondo-lattice metal: Evidence from an optical study

    PubMed Central

    Kovaleva, N. N.; Kugel, K. I.; Bazhenov, A. V.; Fursova, T. N.; Löser, W.; Xu, Y.; Behr, G.; Kusmartsev, F. V.

    2012-01-01

    Magnetic materials are usually divided into two classes: those with localised magnetic moments, and those with itinerant charge carriers. We present a comprehensive experimental (spectroscopic ellipsomerty) and theoretical study to demonstrate that these two types of magnetism do not only coexist but complement each other in the Kondo-lattice metal, Tb2PdSi3. In this material the itinerant charge carriers interact with large localised magnetic moments of Tb(4f) states, forming complex magnetic lattices at low temperatures, which we associate with self-organisation of magnetic clusters. The formation of magnetic clusters results in low-energy optical spectral weight shifts, which correspond to opening of the pseudogap in the conduction band of the itinerant charge carriers and development of the low- and high-spin intersite electronic transitions. This phenomenon, driven by self-trapping of electrons by magnetic fluctuations, could be common in correlated metals, including besides Kondo-lattice metals, Fe-based and cuprate superconductors. PMID:23189239

  14. Keldysh effective action theory for universal physics in spin-(1)/(2) Kondo dots

    NASA Astrophysics Data System (ADS)

    Smirnov, Sergey; Grifoni, Milena

    2013-03-01

    We present a theory for the Kondo spin-(1)/(2) effect in strongly correlated quantum dots. The theory is applicable at any temperature and voltage. It is based on a quadratic Keldysh effective action parametrized by a universal function. We provide a general analytical form for the tunneling density of states through this universal function for which we propose a simple microscopic model. We apply our theory to the highly asymmetric Anderson model with U=∞ and describe its strong-coupling limit, weak-coupling limit, and crossover region within a single analytical expression. We compare our results with a numerical renormalization group in equilibrium and with a real-time renormalization group out of equilibrium and show that the universal shapes of the linear and differential conductance obtained in our theory and in these theories are very close to each other in a wide range of temperatures and voltages. In particular, as in the real-time renormalization group, we predict that at the Kondo voltage the differential conductance is equal to 2/3 of its maximum.

  15. Spin relaxation through Kondo scattering in Cu/Py lateral spin valves

    NASA Astrophysics Data System (ADS)

    Batley, J. T.; Rosamond, M. C.; Ali, M.; Linfield, E. H.; Burnell, G.; Hickey, B. J.

    2015-12-01

    The temperature dependence of the spin diffusion length typically reflects the scattering mechanism responsible for spin relaxation. Within nonmagnetic metals it is reasonable to expect the Elliot-Yafet mechanism to play a role and thus the temperature dependence of the spin diffusion length might be inversely proportional to resistivity. In lateral spin valves, measurements have found that at low temperatures the spin diffusion length unexpectedly decreases. By measuring the transport properties of lateral Py/Cu/Py spin valves, fabricated from Cu with magnetic impurities of <1 ppm and ˜4 ppm, we extract a spin diffusion length which shows this suppression below 30 K only in the presence of the Kondo effect. We have calculated the spin-relaxation rate and isolated the contribution from magnetic impurities. We find the spin-flip probability of a magnetic impurity to be 34%. Our analysis demonstrates the dominant role of Kondo scattering in spin relaxation, even in low concentrations of order 1 ppm, and hence illustrates its importance to the reduction in spin diffusion length observed by ourselves and others.

  16. Heavy-fermion quantum criticality and destruction of the Kondo effect in a nickel oxypnictide.

    PubMed

    Luo, Yongkang; Pourovskii, Leonid; Rowley, S E; Li, Yuke; Feng, Chunmu; Georges, Antoine; Dai, Jianhui; Cao, Guanghan; Xu, Zhu'an; Si, Qimiao; Ong, N P

    2014-08-01

    A quantum critical point arises at a continuous transformation between distinct phases of matter at zero temperature. Studies in antiferromagnetic heavy-fermion materials have revealed that quantum criticality has several classes, with an unconventional type that involves a critical destruction of the Kondo entanglement. To understand such varieties, it is important to extend the materials basis beyond the usual setting of intermetallic compounds. Here we show that a nickel oxypnictide, CeNiAsO, exhibits a heavy-fermion antiferromagnetic quantum critical point as a function of either pressure or P/As substitution. At the quantum critical point, non-Fermi-liquid behaviour appears, which is accompanied by a divergent effective carrier mass. Across the quantum critical point, the low-temperature Hall coefficient undergoes a rapid sign change, suggesting a sudden jump of the Fermi surface and a destruction of the Kondo effect. Our results imply that the enormous materials basis for the oxypnictides, which has been so crucial in the search for high-temperature superconductivity, will also play a vital role in the effort to establish the universality classes of quantum criticality in strongly correlated electron systems.

  17. Heavy-fermion quantum criticality and destruction of the Kondo effect in a nickel oxypnictide

    NASA Astrophysics Data System (ADS)

    Luo, Yongkang; Pourovskii, Leonid; Rowley, S. E.; Li, Yuke; Feng, Chunmu; Georges, Antoine; Dai, Jianhui; Cao, Guanghan; Xu, Zhu'An; Si, Qimiao; Ong, N. P.

    2014-08-01

    A quantum critical point arises at a continuous transformation between distinct phases of matter at zero temperature. Studies in antiferromagnetic heavy-fermion materials have revealed that quantum criticality has several classes, with an unconventional type that involves a critical destruction of the Kondo entanglement. To understand such varieties, it is important to extend the materials basis beyond the usual setting of intermetallic compounds. Here we show that a nickel oxypnictide, CeNiAsO, exhibits a heavy-fermion antiferromagnetic quantum critical point as a function of either pressure or P/As substitution. At the quantum critical point, non-Fermi-liquid behaviour appears, which is accompanied by a divergent effective carrier mass. Across the quantum critical point, the low-temperature Hall coefficient undergoes a rapid sign change, suggesting a sudden jump of the Fermi surface and a destruction of the Kondo effect. Our results imply that the enormous materials basis for the oxypnictides, which has been so crucial in the search for high-temperature superconductivity, will also play a vital role in the effort to establish the universality classes of quantum criticality in strongly correlated electron systems.

  18. A 1Ds ×1Dc Heisenberg-Kondo Lattice compound Nb12O29

    NASA Astrophysics Data System (ADS)

    Pickett, Warren; Lee, Kwan-Woo

    2015-03-01

    Local moments embedded in conducting systems form a rich platform for unusual phases, with phenomena including Kondo, heavy fermion, and non-Fermi liquid physics. Using first principles based methods and the refined crystal structure based on columns of 3 ×4 planar units of NbO6 octahedra, we determine that mixed valent Nb12O29 displays tightly bound local moments forming spin chains along one direction criss-crossed by conducting ``nanowires'' in the perpendicular direction. Just how local moments - very rare for Nb - emerge and coexist with itinerant electrons, an enigma for decades in this system, is elucidated based on the local structure of the NbO6 octahedra and orbital+spin ordering. The resulting 1Ds ×1Dc Heisenberg-Kondo lattice (s=spin, c=charge) picture will be discussed. NRF-2013R1A1A2A10008946 (K.W.L.), DOE DE-FG02-04ER46111 (W.E.P.).

  19. Resonance states and beating pattern induced by quantum impurity scattering in Weyl/Dirac semimetals

    PubMed Central

    Zheng, Shi-Han; Wang, Rui-Qiang; Zhong, Min; Duan, Hou-Jian

    2016-01-01

    Currently, Weyl semimetals (WSMs) are drawing great interest as a new topological nontrivial phase. When most of the studies concentrated on the clean host WSMs, it is expected that the dirty WSM system would present rich physics due to the interplay between the WSM states and the impurities embedded inside these materials. We investigate theoretically the change of local density of states in three-dimensional Dirac and Weyl bulk states scattered off a quantum impurity. It is found that the quantum impurity scattering can create nodal resonance and Kondo peak/dip in the host bulk states, remarkably modifying the pristine spectrum structure. Moreover, the joint effect of the separation of Weyl nodes and the Friedel interference oscillation causes the unique battering feature. We in detail an- alyze the different contribution from the intra- and inter-node scattering processes and present various scenarios as a consequence of competition between them. Importantly, these behaviors are sensitive significantly to the displacement of Weyl nodes in energy or momentum, from which the distinctive fingerprints can be extracted to identify various semimetal materials experimentally by employing the scanning tunneling microscope. PMID:27808262

  20. Resonance states and beating pattern induced by quantum impurity scattering in Weyl/Dirac semimetals

    NASA Astrophysics Data System (ADS)

    Zheng, Shi-Han; Wang, Rui-Qiang; Zhong, Min; Duan, Hou-Jian

    2016-11-01

    Currently, Weyl semimetals (WSMs) are drawing great interest as a new topological nontrivial phase. When most of the studies concentrated on the clean host WSMs, it is expected that the dirty WSM system would present rich physics due to the interplay between the WSM states and the impurities embedded inside these materials. We investigate theoretically the change of local density of states in three-dimensional Dirac and Weyl bulk states scattered off a quantum impurity. It is found that the quantum impurity scattering can create nodal resonance and Kondo peak/dip in the host bulk states, remarkably modifying the pristine spectrum structure. Moreover, the joint effect of the separation of Weyl nodes and the Friedel interference oscillation causes the unique battering feature. We in detail an- alyze the different contribution from the intra- and inter-node scattering processes and present various scenarios as a consequence of competition between them. Importantly, these behaviors are sensitive significantly to the displacement of Weyl nodes in energy or momentum, from which the distinctive fingerprints can be extracted to identify various semimetal materials experimentally by employing the scanning tunneling microscope.

  1. From bad metal to Kondo insulator: temperature evolution of the optical properties of SmB6

    NASA Astrophysics Data System (ADS)

    Tytarenko, A.; Nakatsukasa, K.; Huang, Y. K.; Johnston, S.; van Heumen, E.

    2016-12-01

    The recent rekindling of interest in the mixed valent Kondo insulator SmB6 as candidate for a first correlated topological insulator has resulted in a wealth of new experimental observations. In particular, angle-resolved photoemission experiments have provided completely new insights into the formation of the low temperature Kondo insulating state starting from the high temperature correlated metal. Here, we report detailed temperature and energy dependent measurements of the optical constants of SmB6 in order to provide a detailed study from the point of view of a bulk sensitive spectroscopic probe. We detect a previously unobserved infrared active optical phonon mode, involving the movement of the Sm ions against the boron cages. The changes taking place in the free carrier response with temperature and their connection to changes in optical transitions between different bands are discussed. We find that the free charge density starts to decrease rapidly below approximately 200 K. Below 60 K a small amount of spectral weight begins to accumulate in low lying interband transitions, indicating the formation of the Kondo insulating state; however, the total integrated spectral weight in our experimental window (∼4.35 eV) decreases. This indicates the involvement of a large Coulomb interaction (> 5 eV) in the formation of the Kondo insulator.

  2. Antiferromagnetic Kondo lattice in the layered compound CePd1–xBi₂ and comparison to the superconductor LaPd1–xBi₂

    SciTech Connect

    Han, Fei; Wan, Xiangang; Phelan, Daniel; Stoumpos, Constantinos C.; Sturza, Mihai; Malliakas, Christos D.; Li, Qing'an; Han, Tian-Heng; Zhao, Qingbiao; Chung, Duck Young; Kanatzidis, Mercouri G.

    2015-07-13

    The layered compound CePd1–xBi₂ with the tetragonal ZrCuSi₂-type structure was obtained from excess Bi flux. Magnetic susceptibility data of CePd1–xBi₂ show an antiferromagnetic ordering below 6 K and are anisotropic along the c axis and the ab plane. The anisotropy is attributed to crystal-electric-field (CEF) effects and a CEF model which is able to describe the susceptibility data is given. An enhanced Sommerfeld coefficient γ of 0.191 J mol Ce⁻¹ K⁻² obtained from specific-heat measurement suggests a moderate Kondo effect in CePd1–xBi₂. Other than the antiferromagnetic peak at 6 K, the resistivity curve shows a shoulderlike behavior around 75 K which could be attributed to the interplay between Kondo and CEF effects. Magnetoresistance and Hall-effect measurements suggest that the interplay reconstructs the Fermi-surface topology of CePd1–xBi₂ around 75 K. Electronic structure calculations reveal that the Pd vacancies are important to the magnetic structure and enhance the CEF effects which quench the orbital moment of Ce at low temperatures.

  3. Screened spin-1 and -1/2 Kondo effect in a triangular quantum dot system with interdot Coulomb repulsion

    NASA Astrophysics Data System (ADS)

    Xiong, Yong-Chen; Wang, Wei-Zhong; Luo, Shi-Jun; Yang, Jun-Tao; Huang, Hai-Ming

    2017-03-01

    By means of the numerical renormalization group (NRG) technique, we study the low temperature transport property and the phase transition for a triangular triple quantum dot system, including two centered dots (dot 1 and 2) and one side dot (dot 3). We focus on the effect of interdot repulsion V between two centered dots in a wide range of the interdot hopping tij (i,j = 1,2,3). When the hoppings between the centered dot and the side dot are symmetric, i.e., t13 = t23, and that between two centered dots t12 is small, two centered dots form a spin triplet when V is absent, and a totally screened spin-1 Kondo effect is observed. In this case, one has a spin 1 that is partially screened by the leads as in the usual spin-1 Kondo model, and the remaining spin 1/2 degree of freedom forms a singlet with the side dot. As V is large enough, one of the centered dots is singly occupied, while the other one is empty. The spin-1/2 Kondo effect is found when t13 is small. For large t12, two centered dots form a spin singlet when V = 0, leading to zero conductance. As V is large enough, the spin-1/2 Kondo effect is recovered in the case of small t13. For asymmetric t13≠t23 and small t12, a crossover is found as V increases in comparison with a first order quantum phase transition for the symmetric case. In the regime of large V, the spin-1/2 Kondo effect could also be found when both t13 and t23 are small. We demonstrate the present model is similar to the side-coupled double dot system in some appropriate regimes, and it appears as a possible realization of side-controllable molecular electronics and spintronics devices.

  4. Stabilization of Kondo Semiconductor State by Sb Doping of CeNi1-σSn1+σ and the General Criterion of Its Appearance

    NASA Astrophysics Data System (ADS)

    Spałek, J.; Ślebarski, A.

    2008-07-01

    Semimetallic off-stoichiometric CeNi1-δSn1+δ-xSbx system with δ≈0.06 is shown to transform into a Kondo semiconductor upon the substitution of few percent of Sb for Sn. The full-gap formation is associated with f-electron localization induced by the combined effect of the collective Kondo-singlet formation and the atomic disorder. Namely, the extra valence electrons introduced with the Sb doping (one per Sb atom) contribute additionally to the formation of the collective Kondo spin-singlet state at low temperatures, as seen by a substantial reduction of the magnetic susceptibility. The precise general definition of the Kondo semiconductor is provided and the difference with either the simple band or the Mott-Hubbard insulators is stressed.

  5. Effects on the torsional vibration behavior in the investigation of dental implant osseointegration using resonance frequency analysis: a numerical approach.

    PubMed

    Zhai, Min; Li, Bing; Li, Dehua

    2017-02-07

    Resonance frequency analysis (RFA) methods are widely used to assess implant stability, particularly the Osstell(®) device. The potential effects associated with this method have been discussed in the literature. Torsional RFA (T-RFA), mentioned in our previous study, could represent a new measurement method. The purpose of this study was to simulate T-shaped and Osstell(®) transducer-implant-bone system models; compare their vibration modes and corresponding resonance frequencies; and investigate the effects of their parameters, such as the effective implant length (EIL), bone quality, and osseointegration level, on the torsional resonance frequency (TRF) and bending resonance frequency (BRF) using three-dimensional finite element analysis. Following the finite element model validation, the TRFs and BRFs for three different EILs and four types of bone quality were obtained, and the change rates during 25 degrees of osseointegration were observed. The analysis showed that an increase in the EIL and a decrease in bone quality have less effect on the declination rate of TRFs than on that of BRFs. TRFs are highly sensitive to the stiffness of the implant-bone interface during the healing period. It was concluded that T-RFA has better sensitivity and specificity.

  6. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2–δAs2

    SciTech Connect

    Luo, Yongkang; Ronning, F.; Wakeham, N.; Lu, Xin; Park, Tuson; Xu, Z. -A.; Thompson, J. D.

    2015-10-19

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2–δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 e/formular unit in CeNi2–δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. Here, the small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening.

  7. Shubnikov-de Haas oscillations in the Kondo semimetal CeNiSn

    NASA Astrophysics Data System (ADS)

    Terashima, Taichi; Terakura, Chieko; Uji, Shinya; Aoki, Haruyoshi; Echizen, Yuji; Takabatake, Toshiro

    2001-03-01

    The title compound CeNiSn was once classified as a Kondo insulator. However, recent studies have suggested that the energy gap opening in CeNiSn is a pseudogap with a finite density of states at the Fermi level (see, for example, Refs. 1-3). In the present work, we succeeded in observing Shubnikov-de Haas oscillations in low-temperature magnetoresistance, and thus directly proved that CeNiSn is a semimetal rather than a semiconductor. We discuss experimental results in terms of a hybridization gap picture. References 1. G. Nakamoto et al., J. Phys. Soc. Jpn. 64, 4834 (1995). 2. K. Nakamura et al., Phys. Rev. B 53, 6385 (1996). 3. K. Izawa et al., J. Phys. Soc. Jpn. 65, 3119 (1996).

  8. Quantum phase transition and protected ideal transport in a Kondo chain

    SciTech Connect

    Tsvelik, A. M.; Yevtushenko, O. M.

    2015-11-30

    We study the low energy physics of a Kondo chain where electrons from a one-dimensional band interact with magnetic moments via an anisotropic exchange interaction. It is demonstrated that the anisotropy gives rise to two different phases which are separated by a quantum phase transition. In the phase with easy plane anisotropy, Z2 symmetry between sectors with different helicity of the electrons is broken. As a result, localization effects are suppressed and the dc transport acquires (partial) symmetry protection. This effect is similar to the protection of the edge transport in time-reversal invariant topological insulators. The phase with easy axis anisotropy corresponds to the Tomonaga-Luttinger liquid with a pronounced spin-charge separation. The slow charge density wave modes have no protection against localizatioin.

  9. Low energy properties of the Kondo chain in the RKKY regime

    SciTech Connect

    D. H. Schimmel; Tsvelik, A. M.; Yevtushenko, O. M.

    2016-05-03

    We study the Kondo chain in the regime of high spin concentration where the low energy physics is dominated by the Ruderman–Kittel–Kasuya–Yosida interaction. As has been recently shown (Tsvelik and Yevtushenko 2015 Phys. Rev. Lett. 115 216402), this model has two phases with drastically different transport properties depending on the anisotropy of the exchange interaction. In particular, the helical symmetry of the fermions is spontaneously broken when the anisotropy is of the easy plane type. This leads to a parametrical suppression of the localization effects. In the present paper we substantially extend the previous theory, in particular, by analyzing a competition of forward- and backward- scattering, including into the theory short range electron interactions and calculating spin correlation functions. In conclusion, we discuss applicability of our theory and possible experiments which could support the theoretical findings.

  10. Spiral to ferromagnetic transition in a Kondo lattice model with a double-well potential

    NASA Astrophysics Data System (ADS)

    Caro, R. C.; Franco, R.; Silva-Valencia, J.

    2016-02-01

    Using the density matrix renormalization group method, we study a system of 171Yb atoms confined in a one-dimensional optical lattice. The atoms in the 1So state undergo a double-well potential, whereas the atoms in the 3P0 state are localized. This system is modelled by the Kondo lattice model plus a double-well potential for the free carries. We obtain phase diagrams composed of ferromagnetic and spiral phases, where the critical points always increase with the interwell tunneling parameter. We conclude that this quantum phase transition can be tuned by the double-well potential parameters as well as by the common parameters: local coupling and density.

  11. Kondo temperature when the Fermi level is near a step in the conduction density of states

    NASA Astrophysics Data System (ADS)

    Fernández, J.; Aligia, A. A.; Roura-Bas, P.; Andrade, J. A.

    2017-01-01

    The (111) surface of Cu, Ag, and Au is characterized by a band of surface Shockley states with a constant density of states beginning slightly below the Fermi energy. These states as well as bulk states hybridize with magnetic impurities which can be placed above the surface. We calculate the characteristic low-temperature energy scale, the Kondo temperature TK of the impurity Anderson model, as the bottom of the conduction band Ds crosses the Fermi energy ɛF. We find simple power laws TK≃|Ds-ɛF| η , where η depends on the sign of Ds-ɛF , the ratio between surface and bulk hybridizations with the impurity Δs/Δb , and the ratio between on-site and Coulomb energy Ed/U in the model.

  12. Low energy properties of the Kondo chain in the RKKY regime

    DOE PAGES

    D. H. Schimmel; Tsvelik, A. M.; Yevtushenko, O. M.

    2016-05-03

    We study the Kondo chain in the regime of high spin concentration where the low energy physics is dominated by the Ruderman–Kittel–Kasuya–Yosida interaction. As has been recently shown (Tsvelik and Yevtushenko 2015 Phys. Rev. Lett. 115 216402), this model has two phases with drastically different transport properties depending on the anisotropy of the exchange interaction. In particular, the helical symmetry of the fermions is spontaneously broken when the anisotropy is of the easy plane type. This leads to a parametrical suppression of the localization effects. In the present paper we substantially extend the previous theory, in particular, by analyzing amore » competition of forward- and backward- scattering, including into the theory short range electron interactions and calculating spin correlation functions. In conclusion, we discuss applicability of our theory and possible experiments which could support the theoretical findings.« less

  13. Kondo effect from a Lorentz-violating domain wall description of superconductivity

    NASA Astrophysics Data System (ADS)

    Bazeia, D.; Brito, F. A.; Mota-Silva, J. C.

    2016-11-01

    We extend recent results on domain wall description of superconductivity in an Abelian Higgs model by introducing a particular Lorentz-violating term. The temperature of the system is interpreted through the fact that the soliton following accelerating orbits is a Rindler observer experiencing a thermal bath. We show that this term can be associated with the Kondo effect, that is, the Lorentz-violating parameter is closely related to the concentration of magnetic impurities living on a superconducting domain wall. We also found that the critical temperature decreasing with the impurity concentration as a non-single-valued function, for the case TK

  14. Large, high quality single-crystals of the new Topological Kondo Insulator, SmB6

    PubMed Central

    Hatnean, M. Ciomaga; Lees, M. R.; Paul, D. M. K.; Balakrishnan, G.

    2013-01-01

    SmB6 has recently been predicted to be a Topological Kondo Insulator, the first strongly correlated heavy fermion material to exhibit topological surface states. High quality crystals are necessary to investigate the topological properties of this material. Single crystal growth of the rare earth hexaboride, SmB6, has been carried out by the floating zone technique using a high power xenon arc lamp image furnace. Large, high quality single-crystals are obtained by this technique. The crystals produced by the floating zone technique are free of contamination from flux materials and have been characterised by resistivity and magnetisation measurements. These crystals are ideally suited for the investigation of both the surface and bulk properties of SmB6. PMID:24166216

  15. Suppression of magnetic excitations near the surface of the topological Kondo insulator SmB6

    NASA Astrophysics Data System (ADS)

    Biswas, P. K.; Legner, M.; Balakrishnan, G.; Hatnean, M. Ciomaga; Lees, M. R.; Paul, D. McK.; Pomjakushina, E.; Prokscha, T.; Suter, A.; Neupert, T.; Salman, Z.

    2017-01-01

    We present a detailed investigation of the temperature and depth dependence of the magnetic properties of the three-dimensional topological Kondo insulator SmB6, in particular, near its surface. We find that local magnetic field fluctuations detected in the bulk are suppressed rapidly with decreasing depths, disappearing almost completely at the surface. We attribute the magnetic excitations to spin excitons in bulk SmB6, which produce local magnetic fields of about ˜1.8 mT fluctuating on a time scale of ˜60 ns . We find that the excitonic fluctuations are suppressed when approaching the surface on a length scale of ˜40 -90 nm , accompanied by a small enhancement in static magnetic fields. We associate this length scale to the size of the excitonic state.

  16. Universality and Scaling in a Charge Two-Channel Kondo Device

    NASA Astrophysics Data System (ADS)

    Mitchell, A. K.; Landau, L. A.; Fritz, L.; Sela, E.

    2016-04-01

    We study a charge two-channel Kondo model, demonstrating that recent experiments [Z. Iftikhar et al, Nature (London) 526, 233 (2015)] realize an essentially perfect quantum simulation—not just of its universal physics, but also nonuniversal effects away from the scaling limit. Numerical renormalization group (RG) calculations yield conductance line shapes encoding RG flow to a critical point involving a free Majorana fermion. By mimicking the experimental protocol, the experimental curve is reproduced quantitatively over 9 orders of magnitude, although we show that far greater bandwidth/temperature separation is required to obtain the universal result. Fermi liquid instabilities are also studied: In particular, our exact analytic results for nonlinear conductance provide predictions away from thermal equilibrium, in the regime of existing experiments.

  17. Quantum phase transition and protected ideal transport in a Kondo chain

    DOE PAGES

    Tsvelik, A. M.; Yevtushenko, O. M.

    2015-11-30

    We study the low energy physics of a Kondo chain where electrons from a one-dimensional band interact with magnetic moments via an anisotropic exchange interaction. It is demonstrated that the anisotropy gives rise to two different phases which are separated by a quantum phase transition. In the phase with easy plane anisotropy, Z2 symmetry between sectors with different helicity of the electrons is broken. As a result, localization effects are suppressed and the dc transport acquires (partial) symmetry protection. This effect is similar to the protection of the edge transport in time-reversal invariant topological insulators. The phase with easy axismore » anisotropy corresponds to the Tomonaga-Luttinger liquid with a pronounced spin-charge separation. The slow charge density wave modes have no protection against localizatioin.« less

  18. Interacting topological phases in thin films of topological mirror Kondo insulators

    NASA Astrophysics Data System (ADS)

    Zhang, Rui-Xing; Xu, Cenke; Liu, Chao-Xing

    2016-12-01

    We study interaction effects on thin films of topological mirror Kondo insulators (TMKIs), where the strong interaction is expected to play an important role. Our study has led to the following results: (i) We identify a rich phase diagram of noninteracting TMKIs with different mirror Chern numbers in the monolayer and bilayer thin films; (ii) we obtain the phase diagram with interaction and identify the regimes of interaction parameters to mimic bosonic symmetry-protected topological phases with either gapless bosonic modes or spontaneous mirror symmetry breaking at the boundary; and (iii) for the spontaneous mirror symmetry-breaking boundary, we also study various domain-wall defects between different mirror symmetry-breaking order parameters at the boundary. Our results reveal that the thin-film TMKI serves as an intriguing platform for experimental studies of interacting topological phases.

  19. From tunneling to contact in a magnetic atom: The non-equilibrium Kondo effect

    NASA Astrophysics Data System (ADS)

    Choi, Deung-Jang; Abufager, Paula; Limot, Laurent; Lorente, Nicolás

    2017-03-01

    A low-temperature scanning tunneling microscope was employed to study the differential conductance in an atomic junction formed by an adsorbed Co atom on a Cu(100) surface and a copper-covered tip. A zero-bias anomaly (ZBA) reveals spin scattering off the Co atom, which is assigned to a Kondo effect. The ZBA exhibits a characteristic asymmetric lineshape when electrons tunnel between tip and sample, while upon the tip-Co contact it symmetrizes and broadens. Through density functional theory calculations and the non-equilibrium non-crossing approximation, we show that the lineshape broadening is mainly a consequence of the additional coupling to the tip, while non-equilibrium effects only modify the large-bias tails of the ZBA.

  20. Foundations of heavy-fermion superconductivity: lattice Kondo effect and Mott physics.

    PubMed

    Steglich, Frank; Wirth, Steffen

    2016-08-01

    This article overviews the development of heavy-fermion superconductivity, notably in such rare-earth-based intermetallic compounds which behave as Kondo-lattice systems. Heavy-fermion superconductivity is of unconventional nature in the sense that it is not mediated by electron-phonon coupling. Rather, in most cases the attractive interaction between charge carriers is apparently magnetic in origin. Fluctuations associated with an antiferromagnetic (AF) quantum critical point (QCP) play a major role. The first heavy-fermion superconductor CeCu2Si2 turned out to be the prototype of a larger group of materials for which the underlying, often pressure-induced, AF QCP is likely to be of a three-dimensional (3D) spin-density-wave (SDW) variety. For UBe13, the second heavy-fermion superconductor, a magnetic-field-induced 3D SDW QCP inside the superconducting phase can be conjectured. Such a 'conventional', itinerant QCP can be well understood within Landau's paradigm of order-parameter fluctuations. In contrast, the low-temperature normal-state properties of a few heavy-fermion superconductors are at odds with the Landau framework. They are characterized by an 'unconventional', local QCP which may be considered a zero-temperature 4 f-orbital selective Mott transition. Here, as concluded for YbRh2Si2, the breakdown of the Kondo effect concurring with the AF instability gives rise to an abrupt change of the Fermi surface. Very recently, superconductivity was discovered for this compound at ultra-low temperatures. Therefore, YbRh2Si2 along with CeRhIn5 under pressure provide a natural link between the large group of about fifty low-temperature heavy-fermion superconductors and other families of unconventional superconductors with substantially higher T c, e.g. the doped Mott insulators of the perovskite-type cuprates and the organic charge-transfer salts.

  1. Foundations of heavy-fermion superconductivity: lattice Kondo effect and Mott physics

    NASA Astrophysics Data System (ADS)

    Steglich, Frank; Wirth, Steffen

    2016-08-01

    This article overviews the development of heavy-fermion superconductivity, notably in such rare-earth-based intermetallic compounds which behave as Kondo-lattice systems. Heavy-fermion superconductivity is of unconventional nature in the sense that it is not mediated by electron-phonon coupling. Rather, in most cases the attractive interaction between charge carriers is apparently magnetic in origin. Fluctuations associated with an antiferromagnetic (AF) quantum critical point (QCP) play a major role. The first heavy-fermion superconductor CeCu2Si2 turned out to be the prototype of a larger group of materials for which the underlying, often pressure-induced, AF QCP is likely to be of a three-dimensional (3D) spin-density-wave (SDW) variety. For UBe13, the second heavy-fermion superconductor, a magnetic-field-induced 3D SDW QCP inside the superconducting phase can be conjectured. Such a ‘conventional’, itinerant QCP can be well understood within Landau’s paradigm of order-parameter fluctuations. In contrast, the low-temperature normal-state properties of a few heavy-fermion superconductors are at odds with the Landau framework. They are characterized by an ‘unconventional’, local QCP which may be considered a zero-temperature 4 f-orbital selective Mott transition. Here, as concluded for YbRh2Si2, the breakdown of the Kondo effect concurring with the AF instability gives rise to an abrupt change of the Fermi surface. Very recently, superconductivity was discovered for this compound at ultra-low temperatures. Therefore, YbRh2Si2 along with CeRhIn5 under pressure provide a natural link between the large group of about fifty low-temperature heavy-fermion superconductors and other families of unconventional superconductors with substantially higher T c, e.g. the doped Mott insulators of the perovskite-type cuprates and the organic charge-transfer salts.

  2. Spin-dependent beating patterns in thermoelectric properties: Filtering the carriers of the heat flux in a Kondo adatom system

    NASA Astrophysics Data System (ADS)

    Seridonio, A. C.; Siqueira, E. C.; Franco, R.; Silva-Valencia, J.; Shelykh, I. A.; Figueira, M. S.

    2014-11-01

    We theoretically investigate the thermoelectric properties of a spin-polarized two-dimensional electron gas hosting a Kondo adatom hybridized with a STM tip. Such a setup is treated within the single-impurity Anderson model in combination with the atomic approach for the Green's functions. Due to the spin dependence of the Fermi wave numbers, the electrical and thermal conductances together with thermopower and Lorenz number reveal beating patterns as a function of the STM tip position in the Kondo regime. In particular, by tuning the lateral displacement of the tip with respect to the adatom vicinity, the temperature, and the position of the adatom level, one can change the sign of the Seebeck coefficient through charge and spin. This opens a possibility of the microscopic control of the heat flux analogously to that established for the electrical current.

  3. Quantum phases of the Shastry-Sutherland Kondo lattice: implications for the global phase diagram of heavy-fermion metals.

    PubMed

    Pixley, J H; Yu, Rong; Si, Qimiao

    2014-10-24

    Considerable recent theoretical and experimental effort has been devoted to the study of quantum criticality and novel phases of antiferromagnetic heavy-fermion metals. In particular, quantum phase transitions have been discovered in heavy-fermion compounds with geometrical frustration. These developments have motivated us to study the competition between the Ruderman-Kittel-Kasuya-Yosida and Kondo interactions on the Shastry-Sutherland lattice. We determine the zero-temperature phase diagram as a function of magnetic frustration and Kondo coupling within a slave-fermion approach. Pertinent phases include the valence bond solid and heavy Fermi liquid. In the presence of antiferromagnetic order, our zero-temperature phase diagram is remarkably similar to the global phase diagram proposed earlier based on general grounds. We discuss the implications of our results for the experiments on Yb2Pt2Pb and related compounds.

  4. Two-Channel Kondo Physics due to As Vacancies in the Layered Compound ZrAs1.58 Se0.39

    NASA Astrophysics Data System (ADS)

    Cichorek, T.; Bochenek, L.; Schmidt, M.; Czulucki, A.; Auffermann, G.; Kniep, R.; Niewa, R.; Steglich, F.; Kirchner, S.

    2016-09-01

    We address the origin of the magnetic-field-independent -|A |T1 /2 term observed in the low-temperature resistivity of several As-based metallic systems of the PbFCl structure type. For the layered compound ZrAs1.58 Se0.39 , we show that vacancies in the square nets of As give rise to the low-temperature transport anomaly over a wide temperature regime of almost two decades in temperature. This low-temperature behavior is in line with the nonmagnetic version of the two-channel Kondo effect, whose origin we ascribe to a dynamic Jahn-Teller effect operating at the vacancy-carrying As layer with a C4 symmetry. The pair-breaking nature of the dynamical defects in the square nets of As explains the low superconducting transition temperature Tc≈0.14 K of ZrAs1.58 Se0.39 compared to the free-of-vacancies homologue ZrP1.54 S0.46 (Tc≈3.7 K ). Our findings should be relevant to a wide class of metals with disordered pnictogen layers.

  5. Non-Kondo-like electronic structure in the correlated rare-earth hexaboride YbB6

    DOE PAGES

    Neupane, Madhab; Xu, Su -Yang; Alidoust, Nasser; ...

    2015-01-07

    Here, we present angle-resolved photoemission studies on the rare-earth-hexaboride YbB6, which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB6 exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB6 has three 2D Dirac cone like surface states enclosing the Kramers’s points, while the f orbital that would be relevant for the Kondo mechanism is ~1 eV below the Fermi level. Our first-principles calculation shows that the topological state that we observe inmore » YbB6 is due to an inversion between Yb d and B p bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.« less

  6. Effects of electron-phonon coupling in the Kondo regime of a two-orbital single-molecule junction

    NASA Astrophysics Data System (ADS)

    Vernek, Edson; Iorio, Gisele; Deng, Lili; Ingersent, Kevin; Anda, Enrique

    2012-02-01

    Single-molecule junctions (SMJs) are electronic devices formed by a molecule bridging the gap between two metallic contacts. Despite their apparent simplicity, such systems have attracted much attention for the rich variety of experimentally accessible physics that they display. The spatial confinement of electrons in molecules can lead to collective phenomena such as Coulomb blockade and the Kondo effect, as well as to strong coupling of electrons to molecular vibrations. We explore the interesting interplay of electron-electron and electron-phonon interactions in a model of an SMJ in which the central molecule has two active orbitals. The nonperturbative numerical renormalization group method is used to treat the many-body Kondo physics and electron-phonon coupling on equal footing. Electron-phonon coupling renormalizes the energies and Coulomb interactions of the molecular orbitals. The effects are most pronounced in cases where both molecular orbitals lie close to the Fermi energy of the contacts. Here, a sufficiently strong phonon-assisted inter-orbital tunneling can suppress the Kondo effect and cause a crossover to a phonon-dominated regime having very different electrical transport properties.

  7. Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect

    NASA Astrophysics Data System (ADS)

    Du, Shixuan

    Control over charge and spin states at the single molecule level is crucial not only for a fundamental understanding of charge and spin interactions but also represents a prerequisite for development of molecular electronics and spintronics. In this talk, I will talk about the extended spin distribution in space beyond the central Mn ion, and onto the non-magnetic constituent atoms of the MnPc molecule. This extended spin distribution results in an extended Kondo effect, which can be explained by spin polarization induced by symmetry breaking of the molecular framework, as confirmed by DFT calculations. Measuring the evolution of the Kondo splitting with applied magnetic fields at different atomic sites, we find a spatial variation of the g-factor within a single molecule for the first time. The existence of atomic site-dependent g-factors can be attributed to specific molecular orbitals distributed over the entire molecule. This work not only open up a new opportunity for quantum information recording, but also provide a new route to explore the internal electronic and spin structure of complex molecules, hard to achieve otherwise. (L. W. Liu et al., Phys. Rev. Lett. 2015, 114, 126601. In collaboration with Liwei Liu, Kai Yang, Yuhang Jiang, Li Gao, Qi Liu, Boqun Song, Wende Xiao, Haitao Zhou, Hongjun Gao in CAS, Min Ouyang in MU, and A.H. Castro Neto in SNU.) Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect.

  8. ARPES view on surface and bulk hybridization phenomena in the antiferromagnetic Kondo lattice CeRh2Si2

    PubMed Central

    Patil, S.; Generalov, A.; Güttler, M.; Kushwaha, P.; Chikina, A.; Kummer, K.; Rödel, T. C.; Santander-Syro, A. F.; Caroca-Canales, N.; Geibel, C.; Danzenbächer, S.; Kucherenko, Yu.; Laubschat, C.; Allen, J. W.; Vyalikh, D. V.

    2016-01-01

    The hybridization between localized 4f electrons and itinerant electrons in rare-earth-based materials gives rise to their exotic properties like valence fluctuations, Kondo behaviour, heavy-fermions, or unconventional superconductivity. Here we present an angle-resolved photoemission spectroscopy (ARPES) study of the Kondo lattice antiferromagnet CeRh2Si2, where the surface and bulk Ce-4f spectral responses were clearly resolved. The pronounced 4f 0 peak seen for the Ce terminated surface gets strongly suppressed in the bulk Ce-4f spectra taken from a Si-terminated crystal due to much larger f-d hybridization. Most interestingly, the bulk Ce-4f spectra reveal a fine structure near the Fermi edge reflecting the crystal electric field splitting of the bulk magnetic 4f 15/2 state. This structure presents a clear dispersion upon crossing valence states, providing direct evidence of f-d hybridization. Our findings give precise insight into f-d hybridization penomena and highlight their importance in the antiferromagnetic phases of Kondo lattices. PMID:26987899

  9. Analysis of optical sensing behavior of a novel optical bean-shaped resonator biosensor integrated with MZI configuration

    NASA Astrophysics Data System (ADS)

    Wang, Zhuoran; Yao, Jia; Yuan, Guohui; Yang, Li

    2014-07-01

    A novel optical bean-shaped resonator (BR) biosensor integrated with Mach-Zehnder Interferometer structure based on a silicon-on-isolator platform has been proposed and investigated theoretically and numerically. By characterizing and optimizing the structure, our bean-shaped device exhibits a high extinction ratio over 50 dB and a high Q factor of about 5.46 × 104 in a wide wavelength span. The quasi-free spectral range (FSR) is about 469 nm. The sensitivity of 688.6 nm/refractive index unit (RIU) is achieved for bulk changes of refractive index and the detection range varies from 10-6 to 0.689 RIU. More complex bean-shaped structures can also be cascaded by adding more bending waveguides in BR to obtain wider quasi-FSR range.

  10. Kondo Physics at Interfaces in Metallic Non-Local Spin Transport Devices

    NASA Astrophysics Data System (ADS)

    Leighton, Chris

    2015-03-01

    Despite the maturity of metallic spintronics there remain large gaps in our understanding of spin transport in metals, particularly with injection of spins across ferromagnetic/non-magnetic (FM/NM) interfaces, and their subsequent diffusion and relaxation. Unresolved issues include the limits of applicability of Elliott-Yafet spin relaxation, quantification of the influence of defects, surfaces, and interfaces on spin relaxation at nanoscopic dimensions, and the importance of magnetic and spin-orbit scattering. The non-local spin-valve is an enabling device in this context as, in addition to offering potentially disruptive applications, it allows for the separation of charge and spin currents. One particularly perplexing issue in metallic non-local spin valves is the widely observed non-monotonicity in the T-dependent spin accumulation, where the spin signal actually decreases at low T, in contrast to simple expectations. In this work, by studying an expanded range of FM/NM combinations (encompassing Ni80Fe20, Ni, Fe, Co, Cu, and Al), we demonstrate that this effect is not a property of a given FM or NM, but rather of the FM/NM pair. The non-monotonicity is in fact strongly correlated with the ability of the FM to form a dilute local magnetic moment in the NM. We show that local moments, resulting in this case from the ppm-level tail of the FM/NM interdiffusion profile, suppress the injected spin polarization and diffusion length via a novel manifestation of the Kondo effect, explaining all observations associated with the low T downturn in spin accumulation. We further show: (a) that this effect can be promoted by thermal annealing, at which point the conventional charge transport Kondo effect is simultaneously detected in the NM, and (b) that this suppression in spin accumulation can be quenched, even at interfaces that are highly susceptible to the effect, by insertion of a thin non-moment-supporting interlayer. Important implications for room temperature

  11. Flight Behavior of an Asymmetric Body through Spark Range Experiments Using Roll-Yaw Resonance for Yaw Enhancement

    DTIC Science & Technology

    2015-07-01

    asymmetric mass was placed within the body. This internal asymmetry creates a trim moment and angle of attack that is amplified during free -flight as...attack amplitude in this manner enables analysis of a rich set of flight behaviors. Free -flight experiments were conducted on this flight body in the...8 Fig. 6 Shadowgraph of model during free -flight experiment .........................11 Fig. 7 Angular motion for TRN39362

  12. Reconfigurable optical routers based on Coupled Resonator Induced Transparency resonances.

    PubMed

    Mancinelli, M; Bettotti, P; Fedeli, J M; Pavesi, L

    2012-10-08

    The interferometric coupling of pairs of resonators in a resonator sequence generates coupled ring induced transparency (CRIT) resonances. These have quality factors an order of magnitude greater than those of single resonators. We show that it is possible to engineer CRIT resonances in tapered SCISSOR (Side Coupled Integrated Space Sequence of Resonator) to realize fast and efficient reconfigurable optical switches and routers handling several channels while keeping single channel addressing capabilities. Tapered SCISSORs are fabricated in silicon-on-insulator technology. Furthermore, tapered SCISSORs show multiple-channel switching behavior that can be exploited in DWDM applications.

  13. Behaviorism

    ERIC Educational Resources Information Center

    Moore, J.

    2011-01-01

    Early forms of psychology assumed that mental life was the appropriate subject matter for psychology, and introspection was an appropriate method to engage that subject matter. In 1913, John B. Watson proposed an alternative: classical S-R behaviorism. According to Watson, behavior was a subject matter in its own right, to be studied by the…

  14. Relationship between diffusivity of water molecules inside hydrating tablets and their drug release behavior elucidated by magnetic resonance imaging.

    PubMed

    Kikuchi, Shingo; Onuki, Yoshinori; Kuribayashi, Hideto; Takayama, Kozo

    2012-01-01

    We reported previously that sustained release matrix tablets showed zero-order drug release without being affected by pH change. To understand drug release mechanisms more fully, we monitored the swelling and erosion of hydrating tablets using magnetic resonance imaging (MRI). Three different types of tablets comprised of polyion complex-forming materials and a hydroxypropyl methylcellulose (HPMC) were used. Proton density- and diffusion-weighted images of the hydrating tablets were acquired at intervals. Furthermore, apparent self-diffusion coefficient maps were generated from diffusion-weighted imaging to evaluate the state of hydrating tablets. Our findings indicated that water penetration into polyion complex tablets was faster than that into HPMC matrix tablets. In polyion complex tablets, water molecules were dispersed homogeneously and their diffusivity was relatively high, whereas in HPMC matrix tablets, water molecule movement was tightly restricted within the gel. An optimal tablet formulation determined in a previous study had water molecule penetration and diffusivity properties that appeared intermediate to those of polyion complex and HPMC matrix tablets; water molecules were capable of penetrating throughout the tablets and relatively high diffusivity was similar to that in the polyion complex tablet, whereas like the HPMC matrix tablet, it was well swollen. This study succeeded in characterizing the tablet hydration process. MRI provides profound insight into the state of water molecules in hydrating tablets; thus, it is a useful tool for understanding drug release mechanisms at a molecular level.

  15. Two-dimensional Fermi surfaces in Kondo insulating SmB6

    NASA Astrophysics Data System (ADS)

    Li, Gang

    There has been renewed interest in Samarium Hexaboride, which is a strongly correlated heavy Fermion material. Hybridization between itinerant electrons and localized orbitals lead to an opening of charge gap at low temperature. However, the resistivity of SmB6 does not diverge at low temperature. Former studies suggested that this residual conductance is contributed by various origins. Recent theoretical developments suggest that the particular symmetry of energy bands of SmB6 may host a topologically non-trivial surface state, i.e., a topological Kondo insulator. To probe the Fermiology of the possible metallic surface state, we use sensitive torque magnetometry to detect the de Haas van Alphen (dHvA) effect due to Landau level quantization on flux-grown crystals, down to He-3 temperature and up to 45 Tesla. Our angular and temperature dependent data suggest two-dimensional Fermi Surfaces lie in both crystalline (001) and (101) surface planes of SmB6.

  16. Transport properties of the topological Kondo insulator SmB6 under the irradiation of light

    NASA Astrophysics Data System (ADS)

    Zhu, Guo-Bao; Yang, Hui-Min

    2016-10-01

    In this paper, we study transport properties of the X point in the Brillouin zone of the topological Kondo insulator SmB6 under the application of a circularly polarized light. The transport properties at high-frequency regime and low-frequency regime as a function of the ratio (κ) of the Dresselhaus-like and Rashba-like spin-orbit parameter are studied based on the Floquet theory and Boltzmann equation respectively. The sign of Hall conductivity at high-frequency regime can be reversed by the ratio κ and the amplitude of the light. The amplitude of the current can be enhanced by the ratio κ. Our findings provide a way to control the transport properties of the Dirac materials at low-frequency regime. Project supported by the National Natural Science Foundation of China (Grant Nos. 11504095 and 11447145), the Foundation of Heze University (Grant Nos. XY14B002 and XYPY01), and the Project funded by the Higher Educational Science and Technology Program of Shandong Province, China (Grant No. J15LJ55).

  17. Nonequilibrium spatiotemporal formation of the Kondo screening cloud on a lattice

    NASA Astrophysics Data System (ADS)

    Nuss, Martin; Ganahl, Martin; Arrigoni, Enrico; von der Linden, Wolfgang; Evertz, Hans Gerd

    2015-02-01

    We study the nonequilibrium formation of a spin screening cloud that accompanies the quenching of a local magnetic moment immersed in a Fermi sea at zero temperature. Based on high-precision density matrix renormalization-group results for the interacting single-impurity Anderson model, we discuss the real-time evolution after a quantum quench in the impurity-reservoir hybridization using time-evolving block decimation. We report emergent length and time scales in the spatiotemporal structure of nonlocal correlation functions in the spin and the charge density channel. At equilibrium, our data for the correlation functions and the extracted length scales show good agreement with existing results, as do local time-dependent observables at the impurity. In the time-dependent data, we identify a major signal which defines a "light cone" moving at the Fermi velocity and a ferromagnetic component in its wake. Inside the light cone we find that the structure of the nonequilibrium correlation functions emerges on two time scales. Initially, the qualitative structure of the correlation functions develops rapidly at the lattice Fermi velocity. Subsequently the spin correlations converge to the equilibrium results on a much larger time scale. This process sets a dynamic energy scale, which we identify to be proportional to the Kondo temperature. Outside the light cone we observe two different power-law decays of the correlation functions in space, with time- and interaction-strength-independent exponents.

  18. Competition between heavy fermion and Kondo interaction in isoelectronic A-site-ordered perovskites.

    PubMed

    Meyers, D; Middey, S; Cheng, J-G; Mukherjee, Swarnakamal; Gray, B A; Cao, Yanwei; Zhou, J-S; Goodenough, J B; Choi, Yongseong; Haskel, D; Freeland, J W; Saha-Dasgupta, T; Chakhalian, J

    2014-12-17

    With current research efforts shifting towards the 4d and 5d transition metal oxides, understanding the evolution of the electronic and magnetic structure as one moves away from 3d materials is of critical importance. Here we perform X-ray spectroscopy and electronic structure calculations on A-site-ordered perovskites with Cu in the A-site and the B-sites descending along the ninth group of the periodic table to elucidate the emerging properties as d-orbitals change from partially filled 3d to 4d to 5d. The results show that when descending from Co to Ir, the charge transfers from the cuprate-like Zhang-Rice state on Cu to the t(2g) orbital of the B site. As the Cu d-orbital occupation approaches the Cu(2+) limit, a mixed valence state in CaCu(3)Rh(4)O(12) and heavy fermion state in CaCu(3)Ir(4)O(12) are obtained. The investigated d-electron compounds are mapped onto the Doniach phase diagram of the competing RKKY and Kondo interactions developed for the f-electron systems.

  19. Theory of the electron spin resonance in the heavy fermion metal β-YbAlB4.

    PubMed

    Ramires, Aline; Coleman, Piers

    2014-03-21

    The heavy fermion metal β-YbAlB4 exhibits a bulk room temperature conduction electron spin resonance (ESR) signal which evolves into an Ising-anisotropic f-electron signal exhibiting hyperfine features at low temperatures. We develop a theory for this phenomenon based on the development of resonant scattering off a periodic array of Kondo centers. We show that the hyperfine structure arises from the scattering off the Yb atoms with nonzero nuclear spin, while the constancy of the ESR intensity is a consequence of the presence of crystal electric field excitations of the order of the hybridization strength.

  20. Mechanistic differences in permeation behavior of supersaturated and solubilized solutions of carbamazepine revealed by nuclear magnetic resonance measurements.

    PubMed

    Ueda, Keisuke; Higashi, Kenjirou; Limwikrant, Waree; Sekine, Shuichi; Horie, Toshiharu; Yamamoto, Keiji; Moribe, Kunikazu

    2012-11-05

    A solid dispersion (SPD) of carbamazepine (CBZ) with hydroxypropyl methylcellulose acetate succinate (HPMC-AS) was prepared by the spray drying method. The apparent solubility (37 °C, pH 7.4) of CBZ observed with the SPD was over 3 times higher than the solubility of unprocessed CBZ. The supersaturated solution was stable for 7 days. A higher concentration of CBZ in aqueous medium was also achieved by mixing with Poloxamer 407 (P407), a solubilizing agent. From permeation studies of CBZ using Caco-2 monolayers and dialysis membranes, we observed improved CBZ permeation across the membrane in the supersaturated solution of CBZ/HPMC-AS SPD. On the contrary, the CBZ-solubilized P407 solution exhibited poor permeation by CBZ. The chemical shifts of CBZ on the (1)H NMR spectrum from CBZ/HPMC-AS SPD solution were not altered significantly by coexistence with HPMC-AS. In contrast, an upfield shift of CBZ was observed in the CBZ/P407 solution. The spin-lattice relaxation time (T(1)) over spin-spin relaxation time (T(2)) indicated that the mobility of CBZ in the HPMC-AS solution was much lower than that in water. Meanwhile, the mobility of CBZ in P407 solution was significantly higher than that in water. NMR data indicate that CBZ does not strongly interact with HPMC-AS. CBZ mobility was suppressed due to self-association and microviscosity around CBZ, which do not affect permeation behavior. Most of the CBZ molecules in the CBZ/P407 solution were solubilized in the hydrophobic core of P407, and a few were free to permeate the membrane. The molecular state of CBZ, as evaluated by NMR measurements, directly correlated with permeation behavior.

  1. Field dependence of the magnon dispersion in the Kondo lattice CeCu2 up to 12 T

    NASA Astrophysics Data System (ADS)

    Schedler, R.; Witte, U.; Rotter, M.; Loewenhaupt, M.; Schmidt, W.

    2005-05-01

    CeCu2 can be classified as a Kondo lattice which shows antiferromagnetic (AF) order below TN=3.5K [R. Trump et al., J. Appl. Phys. 69, 4699 (1991)]. The orthorhombic crystal and the simple AF magnetic structure with two magnetic moments in the primitive unit cell requires two magnon modes which are observed in zero and low magnetic fields and well described by spin wave theory. However, at higher fields, at and above 3T, an unexpected, additional magnetic excitation is observed. In contrast to the two low-energy magnon modes, it exhibits a steeper (factor 2) field dependence and a flat dispersion. Its origin is unclear.

  2. Temperature behavior of the conduction electrons in the nitrogen-doped 3C SiC monocrystals as studied by electron spin resonance

    NASA Astrophysics Data System (ADS)

    Savchenko, D.; Kalabukhova, E.; Prokhorov, A.; Lančok, J.; Shanina, B.

    2017-01-01

    The temperature behavior of the electron spin resonance (ESR) spectra of nitrogen donors in n-type bulk 3C SiC monocrystals with (ND - NA) ≈ 1017 cm-3 was studied at T = 10-50 K. The triplet lines due to the hyperfine (hf) interaction with 14N nuclei (I = 1, 99.6%) along with a single line with similar isotropic g values of 2.0050(3) were observed in the ESR spectrum of n-type 3C SiC monocrystals in the temperature interval from 10 to 35 K. The observed reduction of the hf splitting for the nitrogen donor residing cubic position (Nk) in the temperature interval from 15 to 35 K was attributed to the motion narrowing effect of the hf splitting. With further increase of the temperature up to 35 K, only one single line with a Lorentzian lineshape was observed in the ESR spectrum of n-type 3C SiC, which was previously assigned in the literature to the unknown deeper donor center. Based on the temperature behavior of the ESR linewidth, integral intensity, and g-value, we have attributed this signal to the conduction electrons (CEs). The temperature dependence of the CE ESR linewidth was described by an exponential law (Orbach process) with the value of the activation energy ΔE ≈ 40 meV close to the energy separation between 1 s(E) excited energy level and conduction band for nitrogen donors. The nitrogen donor pairs were found in the ESR spectrum of n-type 3C SiC. The electrical characteristics of 3C SiC sample were studied by using the contact-free microwave conductivity. The energy ionization of nitrogen donor Ei = 51.4 meV was obtained from the fitting of the experimental data with the theory.

  3. Repetitive Model of Mild Traumatic Brain Injury Produces Cortical Abnormalities Detectable by Magnetic Resonance Diffusion Imaging (DTI/DKI), Histopathology, and Behavior.

    PubMed

    Yu, Fengshan; Shukla, Dinesh K; Armstrong, Regina C; Marion, Christina M; Radomski, Kryslaine L; Selwyn, Reed G; Dardzinski, Bernard J

    2016-12-20

    Noninvasive detection of mild traumatic brain injury (mTBI) is important for evaluating acute through chronic effects of head injuries, particularly after repetitive impacts. To better detect abnormalities from mTBI, we performed longitudinal studies (baseline, 3, 6, and 42 days) using magnetic resonance diffusion tensor imaging (DTI) and diffusion kurtosis imaging (DKI) in adult mice after repetitive mTBI (r-mTBI; daily × 5) or sham procedure. This r-mTBI produced righting reflex delay and was first characterized in the corpus callosum to demonstrate low levels of axon damage, astrogliosis, and microglial activation, without microhemorrhages. High-resolution DTI-DKI was then combined with post-imaging pathological validation along with behavioral assessments targeted for the impact regions. In the corpus callosum, only DTI fractional anisotropy at 42 days showed significant change post-injury. Conversely, cortical regions under the impact site (M1-M2, anterior cingulate) had reduced axial diffusivity (AD) at all time points with a corresponding increase in axial kurtosis (Ka) at 6 days. Post-imaging neuropathology showed microglial activation in both the corpus callosum and cortex at 42 days after r-mTBI. Increased cortical microglial activation correlated with decreased cortical AD after r-mTBI (r = -0.853; n = 5). Using Thy1-YFP-16 mice to fluorescently label neuronal cell bodies and processes revealed low levels of axon damage in the cortex after r-mTBI. Finally, r-mTBI produced social deficits consistent with the function of this anterior cingulate region of cortex. Overall, vulnerability of cortical regions is demonstrated after mild repetitive injury, with underlying differences of DTI and DKI, microglial activation, and behavioral deficits.

  4. Delayed Methylene Blue Improves Lesion Volume, Multi-Parametric Quantitative Magnetic Resonance Imaging Measurements, and Behavioral Outcome after Traumatic Brain Injury.

    PubMed

    Talley Watts, Lora; Long, Justin Alexander; Boggs, Robert Cole; Manga, Hemanth; Huang, Shiliang; Shen, Qiang; Duong, Timothy Q

    2016-01-15

    Traumatic brain injury (TBI) remains a primary cause of death and disability in both civilian and military populations worldwide. There is a critical need for the development of neuroprotective agents that can circumvent damage and provide functional recovery. We previously showed that methylene blue (MB), a U.S. Food and Drug Administration-grandfathered drug with energy-enhancing and antioxidant properties, given 1 and 3 h post-TBI, had neuroprotective effects in rats. This study aimed to further investigate the neuroprotection of delayed MB treatment (24 h postinjury) post-TBI as measured by lesion volume and functional outcomes. Comparisons were made with vehicle and acute MB treatment. Multi-modal magnetic resonance imaging and behavioral studies were performed at 1 and 3 h and 2, 7, and 14 days after an impact to the primary forelimb somatosensory cortex. We found that delaying MB treatment 24 h postinjury still minimized lesion volume and functional deficits, compared to vehicle-treated animals. The data further support the potential for MB as a neuroprotective treatment, especially when medical teatment is not readily available. MB has an excellent safety profile and is clinically approved for other indications. MB clinical trials on TBI can thus be readily explored.

  5. Identifying non-toxic doses of manganese for manganese-enhanced magnetic resonance imaging to map brain areas activated by operant behavior in trained rats.

    PubMed

    Gálosi, Rita; Szalay, Csaba; Aradi, Mihály; Perlaki, Gábor; Pál, József; Steier, Roy; Lénárd, László; Karádi, Zoltán

    2017-04-01

    Manganese-enhanced magnetic resonance imaging (MEMRI) offers unique advantages such as studying brain activation in freely moving rats, but its usefulness has not been previously evaluated during operant behavior training. Manganese in a form of MnCl2, at a dose of 20mg/kg, was intraperitoneally infused. The administration was repeated and separated by 24h to reach the dose of 40mg/kg or 60mg/kg, respectively. Hepatotoxicity of the MnCl2 was evaluated by determining serum aspartate aminotransferase, alanine aminotransferase, total bilirubin, albumin and protein levels. Neurological examination was also carried out. The animals were tested in visual cue discriminated operant task. Imaging was performed using a 3T clinical MR scanner. T1 values were determined before and after MnCl2 administrations. Manganese-enhanced images of each animal were subtracted from their baseline images to calculate decrease in the T1 value (ΔT1) voxel by voxel. The subtracted T1 maps of trained animals performing visual cue discriminated operant task, and those of naive rats were compared. The dose of 60mg/kg MnCl2 showed hepatotoxic effect, but even these animals did not exhibit neurological symptoms. The dose of 20 and 40mg/kg MnCl2 increased the number of omissions and did not affect the accuracy of performing the visual cue discriminated operant task. Using the accumulated dose of 40mg/kg, voxels with a significant enhanced ΔT1 value were detected in the following brain areas of the visual cue discriminated operant behavior performed animals compared to those in the controls: the visual, somatosensory, motor and premotor cortices, the insula, cingulate, ectorhinal, entorhinal, perirhinal and piriform cortices, hippocampus, amygdala with amygdalohippocampal areas, dorsal striatum, nucleus accumbens core, substantia nigra, and retrorubral field. In conclusion, the MEMRI proved to be a reliable method to accomplish brain activity mapping in correlation with the operant behavior of

  6. The effect of Th substitution and of magnetic field on Kondo semiconducting behaviour in U2Ru2Sn

    NASA Astrophysics Data System (ADS)

    du Plessis, P. de V.; Strydom, A. M.; Troc, R.; Menon, L.

    2001-09-01

    Electrical resistivity, ρ(T), measurements on U2Ru2Sn show typical Kondo semiconducting behaviour, namely a ρ(T)~ln T behaviour at higher temperatures and an activation-like increase in ρ(T) below 20 K which indicates the opening of a small gap in the electronic density of states. The magnetic susceptibility, χ(T), of U2Ru2Sn has a maximum around 180 K which is characteristic of intermediate-valence behaviour. The χ(T) data for U2Ru2Sn have been fitted to the interconfigurational fluctuation model of Sales and Wohlleben giving a value of Tsf* = 155(2) K for the characteristic fluctuation temperature. Substituting as little as 5% Th for U leads to a ρ(T) variation reminiscent of that of a single-ion Kondo metal ρ(T) = ρ(0)[1- (π2/16)(T2/TK2)]. Values of TK = 79(1) and 113(1) K are respectively obtained for alloys with 5% and 10% Th substitution.

  7. Fe Substitution Effect on the High-Field Magnetization in the Kondo Semiconductor CeRu2Al10

    NASA Astrophysics Data System (ADS)

    Kondo, Akihiro; Kindo, Koichi; Nohara, Hiroki; Nakamura, Michio; Tanida, Hiroshi; Sera, Masafumi; Nishioka, Takashi

    2017-02-01

    The magnetization of the Fe substitution system in the Kondo semiconductor CeRu2Al10 was measured in high magnetic fields of up to 72 T with the magnetic field (H) along the a-axis. The magnetization curve indicates that the critical field from the antiferromagnetic (AFM) phase to the paramagnetic one (Hcp) shows an increase from ˜51 (x = 0) to ˜60 T (x = 0.7) owing to the Fe substitution. The Fe concentration dependence of Hcp is similar to that of the magnitude of the energy of the spin gap. The degree of the concave H dependence of the magnetization curve, which is the characteristic feature for H ∥ a in CeT2Al10 (T = Ru, Os), is not strongly enhanced by the Fe substitution. This may be due to the suppression of the strong anisotropy of the hybridization between the conduction band and the localized 4f shell along the a-axis. These results reveal that the spin gap of the present system consists of at least two components, the gap due to the spin (Kondo) singlet formation and the anisotropy gap of the AF magnon.

  8. Magnetic susceptibility of Dirac fermions, Bi-Sb alloys, interacting Bloch fermions, dilute nonmagnetic alloys, and Kondo alloys

    NASA Astrophysics Data System (ADS)

    Buot, Felix A.; Otadoy, Roland E. S.; Rivero, Karla B.

    2017-03-01

    Wide ranging interest in Dirac Hamiltonian is due to the emergence of novel materials, namely, graphene, topological insulators and superconductors, the newly-discovered Weyl semimetals, and still actively-sought after Majorana fermions in real materials. We give a brief review of the relativistic Dirac quantum mechanics and its impact in the developments of modern physics. The quantum band dynamics of Dirac Hamiltonian is crucial in resolving the giant diamagnetism of bismuth and Bi-Sb alloys. Quantitative agreement of the theory with the experiments on Bi-Sb alloys has been achieved, and physically meaningful contributions to the diamagnetism has been identified. We also treat relativistic Dirac fermion as an interband dynamics in uniform magnetic fields. For the interacting Bloch electrons, the role of translation symmetry for calculating the magnetic susceptibility avoids any approximation to second order in the field. The expressions for magnetic susceptibility of dilute nonmagnetic alloys give a firm theoretical foundation of the empirical formulas used in fitting experimental results. The unified treatment of all the above calculations is based on the lattice Weyl-Wigner formulation of discrete phase-space quantum mechanics. For completeness, the magnetic susceptibility of Kondo alloys is also given since Dirac fermions in conduction band and magnetic impurities exhibit Kondo effect.

  9. Light induced suppression of Kondo effect at amorphous LaAlO3/SrTiO3 interface

    NASA Astrophysics Data System (ADS)

    Liu, G. Z.; Qiu, J.; Jiang, Y. C.; Zhao, R.; Yao, J. L.; Zhao, M.; Feng, Y.; Gao, J.

    2016-07-01

    We report photoelectric properties of two-dimensional electron gas (2DEG) at an amorphous LaAlO3/SrTiO3 interface. Under visible light illumination (650 nm), an enhancement of electric conductivity is observed over the temperature range from 2 to 300 K. Particularly, a resistance upturn appearing below 25 K, which is further proved to from the Kondo effect, is suppressed by the 650 nm visible light. From the results of light-assisted Hall measurements, light irradiation increases the carrier mobility rather than carrier density in the Kondo regime. It is suggested that light induces the decoherence effect of localized spin states, hence the electron scattering is weakened and the carrier mobility is improved accordingly. Moreover, the enhancement of electrical conductivity by visible light verifies that in-gap states located in the SrTiO3 side of the interface play an important role in the electrical transport of the amorphous SrTiO3-based oxide 2DEG system. Our results provide deeper insight into the photoinduced effects in the 2DEG system, paving the way for the design of optoelectronic devices based on oxides.

  10. Topological surface states interacting with bulk excitations in the Kondo insulator SmB6 revealed via planar tunneling spectroscopy

    PubMed Central

    Park, Wan Kyu; Sun, Lunan; Noddings, Alexander; Kim, Dae-Jeong; Fisk, Zachary; Greene, Laura H.

    2016-01-01

    Samarium hexaboride (SmB6), a well-known Kondo insulator in which the insulating bulk arises from strong electron correlations, has recently attracted great attention owing to increasing evidence for its topological nature, thereby harboring protected surface states. However, corroborative spectroscopic evidence is still lacking, unlike in the weakly correlated counterparts, including Bi2Se3. Here, we report results from planar tunneling that unveil the detailed spectroscopic properties of SmB6. The tunneling conductance obtained on the (001) and (011) single crystal surfaces reveals linear density of states as expected for two and one Dirac cone(s), respectively. Quite remarkably, it is found that these topological states are not protected completely within the bulk hybridization gap. A phenomenological model of the tunneling process invoking interaction of the surface states with bulk excitations (spin excitons), as predicted by a recent theory, provides a consistent explanation for all of the observed features. Our spectroscopic study supports and explains the proposed picture of the incompletely protected surface states in this topological Kondo insulator SmB6. PMID:27233936

  11. Nuclear Magnetic Resonance as a Probe of Meso-timescale Dynamics: Ion and H2O Behavior at Mineral-H2O Interfaces

    NASA Astrophysics Data System (ADS)

    Bowers, G. M.; Kirkpatrick, R. J.; Singer, J. W.

    2012-12-01

    One of the important meso-scales in geochemistry is the meso-timescale that is characteristic of processes too slow to probe with light spectroscopy but too fast to probe macroscopically. Nuclear magnetic resonance (NMR) spectroscopy is one of the only analytical methods with dynamic sensitivity to motions with correlation times on the 10-9 to 1 s timescales and is thus a uniquely powerful probe of meso-timescale dynamic behavior. Here, we describe the results of several studies exploring the meso-timescale motion of ions and H2O at the mineral-H2O interface of hectorite, a smectite clay mineral.1-3 2H, 23Na, 39K and 43Ca NMR results show that H2O molecules associated with the interface undergo anisotropic reorientation due to proximity to the surface and surface-associated cations. This motion can be described by rotational diffusion of the H2O molecule about its C2 symmetry axis at GHz frequencies combined with hopping of the H2O molecule about the normal to the smectite surface at ~>200 kHz. This model describes well the observed 2H NMR spectra of Na+, K+, and Ca2+ hectorites over a range temperatures between -80°C and 50°C, with the specific range dependent only on the total system H2O content. At temperatures above -20°C, systems with excess H2O with respect to a two-layer hydrate (low-H2O pastes through dilute aqueous suspensions) experience additional dynamic averaging due to H2O exchange between cation hydration shells, surface-sorbed species, and bulk inter-particle water. The extent of 2H averaging due to this exchange mechanism is strongly affected by the total H2O content in the system, the identity of the charge balancing cation, and the temperature. The dynamic averaging mechanisms affecting the cationic NMR resonances in these systems become dominated by diffusional processes at progressively lower temperatures as the hydration energy of the cation increases. These interfacial cation dynamics and binding sites are strongly affected by surface

  12. Manganese-enhanced magnetic resonance imaging (MEMRI) of rat brain after systemic administration of MnCl₂: hippocampal signal enhancement without disruption of hippocampus-dependent behavior.

    PubMed

    Jackson, Stewart J; Hussey, Rosalind; Jansen, Maurits A; Merrifield, Gavin D; Marshall, Ian; MacLullich, Alasdair; Yau, Joyce L W; Bast, Tobias

    2011-01-01

    Manganese (Mn(2+))-enhanced magnetic resonance (MR) imaging (MEMRI) in rodents offers unique opportunities for the longitudinal study of hippocampal structure and function in parallel with cognitive testing. However, Mn(2+) is a potent toxin and there is evidence that it can interfere with neuronal function. Thus, apart from causing adverse peripheral side effects, Mn(2+) may disrupt the function of brain areas where it accumulates to produce signal enhancement and, thereby, Mn(2+) administration may confound cognitive testing. Here, we examined in male adult Lister hooded rats if a moderate systemic dose of MnCl₂ (200 μmol/kg; two intraperitoneal injections of 100 μmol/kg separated by 1 h) that produces hippocampal MR signal enhancement would disrupt hippocampal function. To this end, we used a delayed-matching-to-place (DMP) watermaze task, which requires rapid allocentric place learning and is highly sensitive to interference with hippocampal function. Tested on the DMP task 1 h and 24 h after MnCl₂ injection, rats did not show any impairment in indices of memory performance (latencies, search preference) or any sensorimotor effects. However, MnCl₂ injection caused acute peripheral effects (severe ataxia and erythema, i.e. redness of paws, ears, and nose) which subsided over 30 min. Additionally, rats injected with MnCl₂ showed reduced weight 1 day after injection and failed to reach the normal weight-growth curve of control rats within the 16 days monitored. Our results indicate that 200 μmol/kg MnCl₂ produces hippocampal MR signal enhancement without disrupting hippocampus-dependent behavior on a rapid place learning task, even though attention must be paid to peripheral side effects.

  13. Antiferromagnetic spin correlations and pseudogaplike behavior in Ca(Fe1-xCox)2As2 studied by 75As nuclear magnetic resonance and anisotropic resistivity

    DOE PAGES

    Cui, J.; Roy, B.; Tanatar, M. A.; ...

    2015-11-06

    We report 75As nuclear magnetic resonance (NMR) measurements of single-crystalline Ca(Fe1–xCox)2As2 (x=0.023, 0.028, 0.033, and 0.059) annealed at 350°C for 7 days. From the observation of a characteristic shape of 75As NMR spectra in the stripe-type antiferromagnetic (AFM) state, as in the case of x=0 (TN=170 K), clear evidence for the commensurate AFM phase transition with the concomitant structural phase transition is observed in x=0.023 (TN=106 K) and x=0.028 (TN=53 K). Through the temperature dependence of the Knight shifts and the nuclear spin lattice relaxation rates (1/T1), although stripe-type AFM spin fluctuations are realized in the paramagnetic state as inmore » the case of other iron pnictide superconductors, we found a gradual decrease of the AFM spin fluctuations below a crossover temperature T* that was nearly independent of Co-substitution concentration, and it is attributed to a pseudogaplike behavior in the spin excitation spectra of these systems. The T* feature finds correlation with features in the temperature-dependent interplane resistivity, ρc(T), but not with the in-plane resistivity ρa(T). The temperature evolution of anisotropic stripe-type AFM spin fluctuations is tracked in the paramagnetic and pseudogap phases by the 1/T1 data measured under magnetic fields parallel and perpendicular to the c axis. As a result, based on our NMR data, we have added a pseudogaplike phase to the magnetic and electronic phase diagram of Ca(Fe1–xCox)2As2.« less

  14. LABCOM resonator Phase 3

    SciTech Connect

    Keres, L.J.

    1990-11-01

    The purpose of this project was to develop quartz crystal resonator designs, production processes, and test capabilities for 5-MHz, 6.2-MHz, and 10-MHz resonators for Tactical Miniature Crystal Oscillator (TMXO) applications. GE Neutron Devices (GEND) established and demonstrated the capability to produce and test quartz crystal resonators for use in the TMXO developed by the US Army ERADCOM (now LABCOM). The goals in this project were based on the ERADCOM statement of work. The scope of work indicated that the resonator production facilities for this project would not be completely independent, but that they would be supported in part by equipment and processes in place at GEND used in US Department of Energy (DOE) work. In addition, provisions for production test equipment or or eventual technology transfer costs to a commercial supplier were clearly excluded from the scope of work. The demonstrated technical capability of the deep-etched blank design is feasible and practical. It can be manufactured in quantity with reasonable yield, and its performance is readily predictable. The ceramic flatpack is a very strong package with excellent hermeticity. The four-point mount supports the crystal to reasonable shock levels and does not perturb the resonator's natural frequency-temperature behavior. The package can be sealed with excellent yields. The high-temperature, high-vacuum processing developed for the TMXO resonator, including bonding the piezoid to its mount with conductive polyimide adhesive, is consistent with precision resonator fabrication. 1 fig., 6 tabs.

  15. Mechanical control of spin states in single molecules

    NASA Astrophysics Data System (ADS)

    Parks, J. J.; Champagne, A. R.; Costi, T. A.; Pasupathy, A. N.; Shum, W. W.; Neuscamman, E.; Chan, G. K.-L.; Abruña, H. D.; Ralph, D. C.

    2010-03-01

    We study individual Co(tpy-SH)2 complexes by connecting them within mechanically controllable break-junction devices that allow us to controllably stretch the molecule while measuring its electrical conductance. At low temperature, this molecule produces the Kondo effect, observed as a peak in the conductance at zero bias. We find that as a function of stretching the Kondo peak splits in two, in distinct contrast to behavior observed in spin-1/2 molecules. The temperature dependence of the Kondo signal for the unstretched molecule is in agreement with the scaling prediction for an underscreened S = 1 Kondo effect. The splitting of the Kondo resonance by mechanical stretching can be explained by a spin-orbit-induced lifting of the degeneracy of the S = 1 triplet upon distortion from octahedral symmetry of the Co ion. We observe evidence of the resultant spin anisotropy in the magnetic-field dependence of the Kondo peaks.

  16. Heavy surface state in a possible topological Kondo insulator: Magnetothermoelectric transport on the (011) plane of SmB6

    DOE PAGES

    Luo, Yongkang; Chen, Hua; Dai, Jianhui; ...

    2015-02-25

    Motivated by the high sensitivity to Fermi surface topology and scattering mechanisms in magnetothermoelectric transport, we have measured the thermopower and Nernst effect on the (011) plane of the proposed topological Kondo insulator SmB6. These experiments, together with electrical resistivity and Hall effect measurements, suggest that the (011) plane also harbors a metallic surface with an effective mass on the order of 10–102 m0. The surface and bulk conductances are well distinguished in these measurements and are categorized into metallic and nondegenerate semiconducting regimes, respectively. As a result, electronic correlations play an important role in enhancing scattering and also contributemore » to the heavy surface state.« less

  17. Anomalous Hall effect in L 10-MnAl films with controllable orbital two-channel Kondo effect

    NASA Astrophysics Data System (ADS)

    Zhu, L. J.; Nie, S. H.; Zhao, J. H.

    2016-05-01

    The anomalous Hall effect (AHE) in strongly disordered magnetic systems has been buried in persistent confusion despite its long history. We report the AHE in perpendicularly magnetized L 10-MnAl epitaxial films with a variable orbital two-channel Kondo (2CK) effect arising from the strong coupling of conduction electrons and the structural disorders of two-level systems. The AHE is observed to excellently scale with ρAH/f =a0ρx x 0+b ρxx 2 at high temperatures where phonon scattering prevails. In contrast, significant deviation occurs at low temperatures where the orbital 2CK effect becomes important, suggesting a negative AHE contribution. The deviation of the scaling agrees with the orbital 2CK effect in the breakdown temperatures and deviation magnitudes.

  18. Carrier-mediated Kondo effect and Hall mobility by electrolyte gating in slightly doped anatase TiO2 films

    NASA Astrophysics Data System (ADS)

    Han, Yin-Long; Luo, Zhong-Zhong; Li, Cheng-Jian; Shen, Sheng-Chun; Qu, Guo-Liang; Xiong, Chang-Min; Dou, Rui-Fen; He, Lin; Nie, Jia-Cai

    2014-11-01

    Carrier density (ns) is a crucial parameter that governs the properties of correlated oxides, so the field-effect approach is an ideal tool to investigate the novel physics of the system. Here, the carrier-mediated transport of slightly doped anatase TiO2 epitaxial films were studied by electric double layer transistor (EDLT) gating. The ns has been increased hugely, and concomitantly, the channels of anatase TiO2 films undergo an insulator-metal transition with a decrease in resistivity by almost three orders of magnitude. More fascinating, the Kondo effect depends very strongly on ns, and the Hall mobility could be enhanced about one order of magnitude with increasing ns. This study shows that EDLT gating is a powerful method to stimulate and mediate novel phenomena of correlated oxides.

  19. Crystal structure and anisotropic magnetic properties of new ferromagnetic Kondo lattice compound Ce(Cu,Al,Si)2

    NASA Astrophysics Data System (ADS)

    Maurya, A.; Thamizhavel, A.; Dhar, S. K.; Provino, A.; Pani, M.; Costa, G. A.

    2017-03-01

    Single crystals of the new compound CeCu0.18Al0.24Si1.58 have been grown by high-temperature solution growth method using a eutectic Al-Si mixture as flux. This compound is derived from the binary CeSi2 (tetragonal α-ThSi2-type, Pearson symbol tI12, space group I41/amd) obtained by partial substitution of Si by Cu and Al atoms but showing full occupation of the Si crystal site (8e). While CeSi2 is a well-known valence-fluctuating paramagnetic compound, the CeCu0.18Al0.24Si1.58 phase orders ferromagnetically at TC=9.3 K. At low temperatures the easy-axis of magnetization is along the a-axis, which re-orients itself along the c-axis above 30 K. The presence of hysteresis in the magnetization curve, negative temperature coefficient of resistivity at high temperatures, reduced jump in the heat capacity and a relatively lower entropy released up to the ordering temperature, and enhanced Sommerfeld coefficient (≈100 mJ/mol K2) show that CeCu0.18Al0.24Si1.58 is a Kondo lattice ferromagnetic, moderate heavy fermion compound. Analysis of the high temperature heat capacity data in the paramagnetic region lets us infer that the crystal electric field split doublet levels are located at 178 and 357 K, respectively, and Kondo temperature (8.4 K) is of the order of TC in CeCu0.18Al0.24Si1.58.

  20. Anderson lattice with explicit Kondo coupling revisited: metamagnetism and the field-induced suppression of the heavy fermion state.

    PubMed

    Howczak, Olga; Spałek, Jozef

    2012-05-23

    We apply the extended (statistically consistent, SCA) Gutzwiller-type approach to the periodic Anderson model (PAM) in an applied magnetic field and in the strong-correlation limit. The finite-U corrections are included systematically by transforming the PAM into the form with the Kondo-type interaction and the residual hybridization, both appearing at the same time and on equal footing. This effective Hamiltonian represents the essence of our Anderson-Kondo lattice model. We show that in ferromagnetic phases the low-energy single-particle states are strongly affected by the presence of the applied magnetic field. We also find that for large values of hybridization strength the system enters the so-called locked heavy fermion state introduced earlier. In this state the chemical potential lies in the majority-spin hybridization gap and, as a consequence, the system evolution is insensitive to further increase of the applied field. However, for a sufficiently strong magnetic field, the system transforms from the locked state to the fully spin-polarized phase. This is accompanied by a metamagnetic transition, as well as by a drastic reduction of the effective mass of the quasiparticles. In particular, we observe no effective mass enhancement in the fully polarized state. The findings are in overall agreement with experimental results for the Ce compounds in high magnetic fields. The mass enhancement for the spin-minority electrons may also diminish with the increasing field, unlike for the quasiparticle states in a single narrow band in the same limit of strong correlations.

  1. Optical resonator

    NASA Technical Reports Server (NTRS)

    Taghavi-Larigani, Shervin (Inventor); Vanzyl, Jakob J. (Inventor); Yariv, Amnon (Inventor)

    2006-01-01

    The invention discloses a semi-ring Fabry-Perot (SRFP) optical resonator structure comprising a medium including an edge forming a reflective facet and a waveguide within the medium, the waveguide having opposing ends formed by the reflective facet. The performance of the SRFP resonator can be further enhanced by including a Mach-Zehnder interferometer in the waveguide on one side of the gain medium. The optical resonator can be employed in a variety of optical devices. Laser structures using at least one SRFP resonator are disclosed where the resonators are disposed on opposite sides of a gain medium. Other laser structures employing one or more resonators on one side of a gain region are also disclosed.

  2. Temperature dependent behavior of localized and delocalized electrons in nitrogen-doped 6H SiC crystals as studied by electron spin resonance

    SciTech Connect

    Savchenko, D.; Kalabukhova, E.; Shanina, B.; Kiselov, V.; Cichoň, S.; Honolka, J.; Mokhov, E.

    2016-01-28

    We have studied the temperature behavior of the electron spin resonance (ESR) spectra of nitrogen (N) donors in n-type 6H SiC crystals grown by Lely and sublimation sandwich methods (SSM) with donor concentration of 10{sup 17 }cm{sup −3} at T = 60–150 K. A broad signal in the ESR spectrum was observed at T ≥ 80 K with Lorentzian lineshape and g{sub ||} = 2.0043(3), g{sub ⊥} = 2.0030(3), which was previously assigned in the literature to the N donors in the 1s(E) excited state. Based on the analysis of the ESR lineshape, linewidth and g-tensor we attribute this signal to the conduction electrons (CE). The emergence of the CE ESR signal at T > 80 K was explained by the ionization of electrons from the 1s(A{sub 1}) ground and 1s(E) excited states of N donors to the conduction band while the observed reduction of the hyperfine (hf) splitting for the N{sub k1,k2} donors with the temperature increase is attributed to the motional narrowing effect of the hf splitting. The temperature dependence of CE ESR linewidth is described by an exponential law (Orbach process) with the activation energy corresponding to the energy separation between 1s(A{sub 1}) and 1s(E) energy levels for N residing at quasi-cubic sites (N{sub k1,k2}). The theoretical analysis of the temperature dependence of microwave conductivity measured by the contact-free method shows that due to the different position of the Fermi level in two samples the ionization of free electrons occurs from the energy levels of N{sub k1,k2} donors in Lely grown samples and from the energy level of N{sub h} residing at hexagonal position in 6H SiC grown by SSM.

  3. Acoustic detection of microbubble resonance

    NASA Astrophysics Data System (ADS)

    Thomas, D. H.; Looney, P.; Steel, R.; Pelekasis, N.; McDicken, W. N.; Anderson, T.; Sboros, V.

    2009-06-01

    Large numbers of acoustic signals from single lipid-shelled Definity® microbubbles have been measured using a calibrated microacoustic system and a two population response observed. Theoretical results based on the Mooney-Rivlin strain softening shell model have been used to identify these populations as primary resonant and off-primary resonant scatter. An experimentally measured size distribution was used to provide the initial resting radius for the simulations, and the responses agree well with the experimental data. In this way, the primary resonant or off-primary resonant behavior of a microbubble can be studied, with potential benefits to both signal processing techniques and microbubble manufacture.

  4. Hydro-acoustic resonance behavior in presence of a precessing vortex rope: observation of a lock-in phenomenon at part load Francis turbine operation

    NASA Astrophysics Data System (ADS)

    Favrel, A.; Landry, C.; Müller, A.; Yamamoto, K.; Avellan, F.

    2014-03-01

    Francis turbines operating at part load condition experience the development of a cavitating helical vortex rope in the draft tube cone at the runner outlet. The precession movement of this vortex rope induces local convective pressure fluctuations and a synchronous pressure pulsation acting as a forced excitation for the hydraulic system, propagating in the entire system. In the draft tube, synchronous pressure fluctuations with a frequency different to the precession frequency may also be observed in presence of cavitation. In the case of a matching between the precession frequency and the synchronous surge frequency, hydro-acoustic resonance occurs in the draft tube inducing high pressure fluctuations throughout the entire hydraulic system, causing torque and power pulsations. The risk of such resonances limits the possible extension of the Francis turbine operating range. A more precise knowledge of the phenomenon occurring at such resonance conditions and prediction capabilities of the induced pressure pulsations needs therefore to be developed. This paper proposes a detailed study of the occurrence of hydro-acoustic resonance for one particular part load operating point featuring a well-developed precessing vortex rope and corresponding to 64% of the BEP. It focuses particularly on the evolution of the local interaction between the pressure fluctuations at the precession frequency and the synchronous surge mode passing through the resonance condition. For this purpose, an experimental investigation is performed on a reduced scale model of a Francis turbine, including pressure fluctuation measurements in the draft tube and in the upstream piping system. Changing the pressure level in the draft tube, resonance occurrences are highlighted for different Froude numbers. The evolution of the hydro-acoustic response of the system suggests that a lock-in effect between the excitation frequency and the natural frequency may occur at low Froude number, inducing a hydro

  5. Upper critical field and Kondo effects in Fe(Te0.9Se0.1) thin films by pulsed field measurements

    DOE PAGES

    Salamon, Myron B.; Cornell, Nicholas; Jaime, Marcelo; ...

    2016-02-10

    The transition temperatures of epitaxial films of Fe(Te0:9Se0:1) are remarkably insensitive to applied magnetic field, leading to predictions of upper critical fields Bc2(T = 0) in excess of 100 T. Using pulsed magnetic fields, we find Bc2(0) to be on the order of 45 T, similar to values in bulk material and still in excess of the paramagnetic limit. The same films show strong magnetoresistance in fields above Bc2(T), consistent with the observed Kondo minimum seen above Tc. Fits to the temperature dependence in the context of the WHH model, using the experimental value of the Maki parameter, require anmore » effective spin-orbit relaxation parameter of order unity. Lastly, we suggest that Kondo localization plays a similar role to spin-orbit pair breaking in making WHH fits to the data.« less

  6. Drastic changes in electronic properties of Kondo semiconductor CeRu2Al10 induced by Rh doping: Anisotropic transport properties in the antiferromagnetic ordered state

    NASA Astrophysics Data System (ADS)

    Tanida, H.; Nohara, H.; Nakagawa, F.; Yoshida, K.; Sera, M.; Nishioka, T.

    2016-10-01

    Electrical resistivity (ρ ), thermopower, and specific heat measurements have been performed on the novel Kondo semiconductor Ce (Ru1-xRhx) 2Al10 (x =0 , 0.02, 0.03, and 0.05), which has been attracting a great deal of interest due to an unusual antiferromagnetic (AFM) order below T0, in order to clarify the Rh doping effect on the anisotropy of the electronic properties in the ordered state. In CeRu2Al10 , ρ shows an anisotropic increase below T0 independently of the electric current direction. We propose the existence of two different mechanisms to explain the anisotropic increase of ρ . One is an isotropic charge gap which enhances ρ below T0 isotropically, although its origin is not known at present. The other is an anisotropic suppression of ρ which originates from the anisotropic c-f hybridization and is largest along the orthorhombic a axis. By the Rh doping, the anisotropic temperature dependence of ρ below T0 is drastically changed. For I ∥b , the increase is almost completely suppressed and a metallic-like behavior is observed, whereas it is small and isotropic for I ∥a and c . From these results, we propose that as a result of the destruction of the spin-gap excitation by the Rh doping, a metallic-like electronic state is formed along the b axis and the small isotropic charge gap is opened in the a c plane. By taking into account the present results and the still high T0 even in x =0.05 , we conclude that the AFM order in the Rh-doped CeRu2Al10 should be viewed as unusual as the AFM order in CeRu2Al10 although the localized character of the Ce-4 f electron is apparently enhanced by the Rh doping. We have also examined the evolution of the AFM ordered state from x =0 to x =0.05 , where the AFM ordered moment (mAF) is aligned along the c axis in x =0 and a axis in x =0.05 . From the results of those experiments in magnetic field, we have revealed that the spin reorientation from mAF∥c to mAF∥a takes place quite abruptly just at xc˜0

  7. Nonlinear resonance

    NASA Astrophysics Data System (ADS)

    Kevorkian, J.

    This report discusses research in the area of slowly varying nonlinear oscillatory systems. Some of the topics discussed are as follows: adiabatic invariants and transient resonance in very slowly varying Hamiltonian systems; sustained resonance in very slowly varying Hamiltonian systems; free-electron lasers with very slow wiggler taper; and bursting oscillators.

  8. Nonlinear resonance

    NASA Astrophysics Data System (ADS)

    Kevorkian, J.; Pernarowski, Mark; Bosley, David L.

    1990-04-01

    The subjects discussed are: transient and sustained resonance for systems with very slowly varying parameters; free electron lasers with very slow wiggler taper; and bursting oscillations in biological systems. Plans are discussed for: FEL applications; transient and sustained resonance; and bursting oscillations.

  9. The Kondo problem. II. Crossover from asymptotic freedom to infrared slavery

    NASA Astrophysics Data System (ADS)

    Schlottmann, P.

    1982-04-01

    In the preceding paper we transformed the s-d Hamiltonian onto a resonance level with a large perturbation and derived the scaling equations for the vertices, the invariant coupling, and the resonance width. The scaling equations are integrated under the assumption that the energy dependence of the resonance width can be neglected. The transcendental equation obtained in this way for the renormalized resonance width is solved in the relevant limits and allows a calculation of the static and dynamical susceptibility. At high temperatures the perturbation expansion for the relaxation rate and the susceptibility is reproduced up to third order in Jρ. At low temperatures the lifetime and χ0 remain finite and vary according to a Fermi-liquid theory. The approximation scheme interpolates in this way between the asymptotic freedom and the infrared slavery, yielding a smooth crossover. The present results are in quantitative agreement with previous ones obtained with the relaxation-kernel method by Götze and Schlottmann. The advantages and drawbacks of the method are discussed. The calculation of the dynamical susceptibility is extended to nonzero external magnetic fields. The quasielastic peak of χ''(ω)ω is suppressed at low temperatures and large magnetic fields and shoulders develop at ω=+/-B.

  10. Observation of a non-Kondo-like topological insulator state in the correlated rare-earth hexaboride YbB6

    NASA Astrophysics Data System (ADS)

    Neupane, Madhab; Xu, S.-Y.; Alidoust, N.; Bian, G.; Liu, C.; Belopolski, I.; Chang, T.-R.; Jeng, H. T.; Durakiewicz, T.; Lin, H.; Bansil, A.; Kim, D. J.; Fisk, Z.; Hasan, M. Z.

    2015-03-01

    We present angle-resolved photoemission studies on the rare-earth hexaboride YbB6, which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB6 exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB6 has three 2D Dirac cone surface states enclosing the Kramers' points, while the f - orbital which would be relevant for the Kondo mechanism is about 1 eV below the Fermi level. Our first-principles calculation shows that the topological state which we observe in YbB6 is due to an inversion between Yb d and B p bands. I will also present some of our recent results on other member of hexaborides. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials. The work at Princeton and Princeton-led synchrotron-based ARPES measurements is supported by U.S. DOE DE-FG-02-05ER46200.

  11. Kondo screening and spin excitation in few-layer CoPc molecular assembly stacking on Pb(111) surface: A DFT+HEOM study

    NASA Astrophysics Data System (ADS)

    Wang, Yu; Zheng, Xiao; Yang, Jinlong

    2016-10-01

    Transition metal phthalocyanine molecules adsorbed on a metal substrate exhibit rich spin-related phenomena such as magnetic anisotropy, spin excitation, and Kondo effect. In this work, we investigate theoretically few-layer cobalt phthalocyanine (CoPc) molecular assembly stacking on Pb(111) surface with the use of a combined density functional theory (DFT) and hierarchical equations of motion (HEOM) approach. Calculation results indicate that the local spin properties of CoPc/Pb(111) composites depend critically on the number of adsorption layers. The first layer of CoPc on the Pb(111) surface serves as a spin-insulating buffer, while the CoPc molecules in the second layer exhibit spin-1/2 Kondo effect with a Kondo temperature of about 22 K. In a triple-layer CoPc assembly stacking on Pb(111), the antiferromagnetic coupling between the second and third layers leads to local spin-flip excitations under finite bias voltages, which gives rise to characteristic signatures in the differential conductance spectra. The DFT+HEOM approach thus provides a practical means for investigating the local electronic and spin properties of two-dimensional molecular assemblies adsorbed on the metal surface. The insights obtained from the first-principles based simulations could be useful for experimental manipulation or design of magnetic composite systems.

  12. Indications of a Quantum Critical Point in Bi2Sr2CaCu2O8+δ Using a Local Kondo Effect

    NASA Astrophysics Data System (ADS)

    Calleja, Eduardo; Dai, Jixia; Arnold, Gerald; Gu, Genda; McElroy, Kyle

    2014-03-01

    A complete understanding of the complex phase diagrams that are present in high temperature superconductors remains elusive. While there is an overwhelming amount of experimental data on the existence and interplay of the phases present in high Tc superconductors from local probes, much of the existing data only looks at the charge degree of freedom of the material. By substituting Fe atoms for Cu atoms in the CuO plane of Bi2Sr2CaCu2O8+δ (Bi2212), we gain the ability to access the spin degree of freedom since the Fe atoms retain their magnetization below the superconducting transition temperature. This leads to a local Kondo effect which can be observed using Spectroscopic-Imaging Scanning Tunneling Microscopy (SI-STM) and the local Kondo temperature can be extracted from spectra via a theoretical model. We show that the examination of this local Kondo temperature across local and sample average doping leads to the observation of a change in the quasiparticle spin degree of freedom at a quantum critical point (QCP) with a nominal hole doping of roughly 0.22, in agreement with other probes. The observation of the QCP in Bi2212 with this new method to access the spin degree of freedom helps to unravel some of the mystery behind the complex phase diagram of Bi2212.

  13. Acoustic Resonators

    NASA Astrophysics Data System (ADS)

    Greenslade, Thomas B.

    2012-11-01

    Recently my collection of historical physics teaching apparatus was given a group of 19th-century tuning forks on resonant boxes. Figure 1 shows the smallest fork sitting on the largest one. The large tuning fork oscillates at 128 Hz and has a resonator that is 57.9 cm long. The small fork has a frequency 10 times higher, but its resonator has a length of 11.0 cm instead of the 5.8 cm that simple scaling would suggest. How is this possible?

  14. Julius Edgar Lilienfeld Prize: Lilienfeld Prize Lecture: Emergent Behavior in Quantum Matter

    NASA Astrophysics Data System (ADS)

    Pines, David

    We live in an emergent universe in which interactions between the basic building blocks of matter and their environment give rise to unpredicted and unexpected emergent behavior at every scale. As physicists we seek to identify the organizing principles responsible for that behavior, construct soluble models that incorporate these, and explain experiment. In this lecture, I illustrate this approach to understanding emergent behavior in quantum matter through three examples: collective modes in electron, helium, and nuclear liquids; the emergence of superconductivity in conventional and unconventional superconductors, nuclei, and neutron stars; and the emergence of heavy electrons in Kondo lattice materials.

  15. Unusual Kondo-hole effect and crystal-field frustration in Nd-doped CeRhIn5

    DOE PAGES

    Rosa, Priscila Ferrari Silveira; Oostra, Aaron; Thompson, Joe David; ...

    2016-07-05

    In this research, we investigate single crystals of Ce1₋xNdxRhIn5 by means of x-ray-diffraction, microprobe, magnetic susceptibility, heat capacity, and electrical resistivity measurements. Our data reveal that the antiferromagnetic transition of CeRhIn5, at Tmore » $$Ce\\atop{N}$$=3.8 K, is linearly suppressed with xNd. We associate this effect with the presence of a “Kondo hole” created by Nd substitution. The extrapolation of T$$Ce\\atop{N}$$ to zero temperature, however, occurs at xc~0.3, which is below the two-dimensional percolation limit found in Ce1₋xLaxRhIn5. This result strongly suggests the presence of a crystal-field induced magnetic frustration. Near xNd~0.2, the Ising antiferromagnetic order from Nd3+ ions is stabilized and T$$Nd\\atop{N}$$ increases up to 11 K in NdRhIn5. Finally, our results shed light on the effects of magnetic doping in heavy-fermion antiferromagnets and stimulate the study of such systems under applied pressure.« less

  16. The Effect of the Berry Phase on the Quantum Critical Properties of the Bose-Fermi Kondo model

    NASA Astrophysics Data System (ADS)

    Kirchner, Stefan; Si, Qimiao

    2006-03-01

    The theory of the quantum critical point of a T=0 transition is traditionally formulated in terms of a quantum-to-classical mapping, leading to a theory of its classical counterpart in elevated dimensions. Recently, it has been shown that this mapping breaks down in an SU(N)xSU(N/2) Bose-Fermi Kondo model (BFKM) [1], a BFKM with Ising anisotropy [2] and the spin-boson model [3]. Here we report the Quantum Monte Carlo results for the scaling properties of the quantum critical point of the BFKM with Ising anisotropy. In addition, using the Lagrangian formulation of the BFKM, we study the critical properties in the presence and absence of the spin Berry phase term. The results of the two cases are compared with the numerical results.[1] L. Zhu, S. Kirchner, Q. Si, and A. Georges, Phys. Rev. Lett. 93,267201 (2004). [2] M. Glossop and K. Ingersent, Phys. Rev. Lett. 95, 067202 (2005). [3] M. Vojta, N-H Tong, and R. Bulla, Phys. Rev. Lett. 94, 070604 (2005).

  17. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6.

    PubMed

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X C; Zhang, Chi; Shi, Jing; Han, Wei

    2016-11-11

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin-momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin-momentum locking property of surface states of SmB6.

  18. Three-dimensional bulk electronic structure of the Kondo lattice CeIn3 revealed by photoemission

    PubMed Central

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Liu, Qin; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Liu, Yu; Song, Haifeng; Zhang, Zhengjun; Lai, Xinchun

    2016-01-01

    We show the three-dimensional electronic structure of the Kondo lattice CeIn3 using soft x-ray angle resolved photoemission spectroscopy in the paramagnetic state. For the first time, we have directly observed the three-dimensional topology of the Fermi surface of CeIn3 by photoemission. The Fermi surface has a complicated hole pocket centred at the Γ-Z line and an elliptical electron pocket centred at the R point of the Brillouin zone. Polarization and photon-energy dependent photoemission results both indicate the nearly localized nature of the 4f electrons in CeIn3, consistent with the theoretical prediction by means of the combination of density functional theory and single-site dynamical mean-field theory. Those results illustrate that the f electrons of CeIn3, which is the parent material of CeMIn5 compounds, are closer to the localized description than the layered CeMIn5 compounds. PMID:27641364

  19. Three-dimensional bulk electronic structure of the Kondo lattice CeIn3 revealed by photoemission

    NASA Astrophysics Data System (ADS)

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Liu, Qin; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Liu, Yu; Song, Haifeng; Zhang, Zhengjun; Lai, Xinchun

    2016-09-01

    We show the three-dimensional electronic structure of the Kondo lattice CeIn3 using soft x-ray angle resolved photoemission spectroscopy in the paramagnetic state. For the first time, we have directly observed the three-dimensional topology of the Fermi surface of CeIn3 by photoemission. The Fermi surface has a complicated hole pocket centred at the Γ-Z line and an elliptical electron pocket centred at the R point of the Brillouin zone. Polarization and photon-energy dependent photoemission results both indicate the nearly localized nature of the 4f electrons in CeIn3, consistent with the theoretical prediction by means of the combination of density functional theory and single-site dynamical mean-field theory. Those results illustrate that the f electrons of CeIn3, which is the parent material of CeMIn5 compounds, are closer to the localized description than the layered CeMIn5 compounds.

  20. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    NASA Astrophysics Data System (ADS)

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X. C.; Zhang, Chi; Shi, Jing; Han, Wei

    2016-11-01

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin-momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin-momentum locking property of surface states of SmB6.

  1. Interplay of atomic randomness and Kondo effect in disordered metallic conductor La2NiSi3

    NASA Astrophysics Data System (ADS)

    Gnida, Daniel; Szlawska, Maria; Swatek, Przemysław; Kaczorowski, Dariusz

    2016-11-01

    A polycrystalline sample of La2NiSi3 was investigated by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity and magnetoresistivity measurements. The compound was basically characterized as a Pauli paramagnet with metallic-like electrical conductivity, notably reduced in magnitude and weakly temperature dependent, as is usually observed for atomically disordered systems. Furthermore, the experimental data revealed the presence of a small amount of paramagnetic impurities. As a result, the low-temperature electrical resistivity in La2NiSi3 was found to be governed by both quantum corrections due to electron-electron interactions (ρ ˜ {{T}1/2} contribution) and spin-flip Kondo scattering (ρ ˜ log T contribution). The presence of paramagnetic impurities led to an increase in s-electron spin splitting due to the s-d interactions, manifested by a B 1/2 dependence of the magnetoresistivity, anomalously observed in the present study for thermal energy being larger than the Zeeman splitting energy {{k}\\text{B}}T>g{μ\\text{B}}B .

  2. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    PubMed Central

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X. C.; Zhang, Chi; Shi, Jing; Han, Wei

    2016-01-01

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin–momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin–momentum locking property of surface states of SmB6. PMID:27834378

  3. Emergent heavy fermion behavior at the Wigner-Mott transition.

    PubMed

    Merino, Jaime; Ralko, Arnaud; Fratini, Simone

    2013-09-20

    We study charge ordering driven by Coulomb interactions on triangular lattices relevant to the Wigner-Mott transition in two dimensions. Dynamical mean-field theory reveals the pinball liquid phase, a charge ordered metallic phase containing quasilocalized (pins) coexisting with itinerant (balls) electrons. Based on an effective periodic Anderson model for this phase, we find an antiferromagnetic Kondo coupling between pins and balls and strong quasiparticle renormalization. Non-Fermi liquid behavior can occur in such charge ordered systems due to the spin-flip scattering of itinerant electrons off the pins in analogy with heavy fermion compounds.

  4. Multiquark resonances

    DOE PAGES

    Esposito, A.; Pilloni, A.; Polosa, Antonio D.

    2016-12-02

    Multiquark resonances are undoubtedly experimentally observed. The number of states and the amount of details on their properties have been growing over the years. It is very recent the discovery of two pentaquarks and the confirmation of four tetraquarks, two of which had not been observed before. We mainly review the theoretical understanding of this sector of particle physics phenomenology and present some considerations attempting a coherent description of the so called X and Z resonances. The prominent problems plaguing theoretical models, like the absence of selection rules limiting the number of states predicted, motivate new directions in model building.more » Lastly, data are reviewed going through all of the observed resonances with particular attention to their common features and the purpose of providing a starting point to further research.« less

  5. Multiquark resonances

    SciTech Connect

    Esposito, A.; Pilloni, A.; Polosa, Antonio D.

    2016-12-02

    Multiquark resonances are undoubtedly experimentally observed. The number of states and the amount of details on their properties have been growing over the years. It is very recent the discovery of two pentaquarks and the confirmation of four tetraquarks, two of which had not been observed before. We mainly review the theoretical understanding of this sector of particle physics phenomenology and present some considerations attempting a coherent description of the so called X and Z resonances. The prominent problems plaguing theoretical models, like the absence of selection rules limiting the number of states predicted, motivate new directions in model building. Lastly, data are reviewed going through all of the observed resonances with particular attention to their common features and the purpose of providing a starting point to further research.

  6. Multiquark resonances

    NASA Astrophysics Data System (ADS)

    Esposito, A.; Pilloni, A.; Polosa, A. D.

    2017-01-01

    Multiquark resonances are undoubtedly experimentally observed. The number of states and the amount of details on their properties have been growing over the years. It is very recent the discovery of two pentaquarks and the confirmation of four tetraquarks, two of which had not been observed before. We mainly review the theoretical understanding of this sector of particle physics phenomenology and present some considerations attempting a coherent description of the so called X and Z resonances. The prominent problems plaguing theoretical models, like the absence of selection rules limiting the number of states predicted, motivate new directions in model building. Data are reviewed going through all of the observed resonances with particular attention to their common features and the purpose of providing a starting point to further research.

  7. Laser Resonator

    NASA Technical Reports Server (NTRS)

    Harper, L. L. (Inventor)

    1983-01-01

    An optical resonator cavity configuration has a unitary mirror with oppositely directed convex and concave reflective surfaces disposed into one fold and concertedly reversing both ends of a beam propagating from a laser rod disposed between two total internal reflection prisms. The optical components are rigidly positioned with perpendicularly crossed virtual rooflines by a compact optical bed. The rooflines of the internal reflection prisms, are arranged perpendicularly to the axis of the laser beam and to the optical axes of the optical resonator components.

  8. Parity crossings of Shiba states and Majorana-like zero bias anomalies in hybrid superconductor-normal nanowire systems with quantum dot behavior

    NASA Astrophysics Data System (ADS)

    Aguado, Ramon; Zitko, Rok; Lopez, Rosa; Lim, Jong Soo

    2015-03-01

    Although recent experiments with semiconducting nanowires are partially consistent with the the existence of Majorana bound states (MBS) at normal-superconductor junctions, other mechanisms cannot be completely ruled out. In this talk, I will focus on short nanowires with quantum dot behavior and discuss the magnetic field dependence of Shiba states as well as novel Kondo features induced by the weak coupling to a normal lead. Our results are based on the phase diagram of an Anderson impurity in contact with superconducting and normal-state leads. This phase diagram is obtained by means of the numerical renormalization group technique and is valid for arbitrary ratio of the superconducting gap to the Kondo temperature. Overall, we find a very rich behavior of spectral functions with zero-bias anomalies which can emerge irrespective of whether the ground state is a doublet or a singlet. This phenomenology originates from crossings of the ground state fermionic parity and mimics that of MBS.

  9. Autostereogram resonators

    NASA Astrophysics Data System (ADS)

    Leavey, Sean; Rae, Katherine; Murray, Adam; Courtial, Johannes

    2012-09-01

    Autostereograms, or "Magic Eye" pictures, are repeating patterns designed to give the illusion of depth. Here we discuss optical resonators that create light patterns which, when viewed from a suitable position by a monocular observer, are autostereograms of the three-dimensional shape of one of the mirror surfaces.

  10. Behavior of Small-Scale Density Fluctuations in Discharges with Off-Axis Electron-Cyclotron Resonance Heating in the T-10 Tokamak

    SciTech Connect

    Shelukhin, D.A.; Vershkov, V.A.; Razumova, K.A.

    2005-12-15

    In experiments on off-axis electron-cyclotron resonance heating in the T-10 tokamak, a steep gradient of the electron temperature was observed to form for a short time at a relative radius of {rho} {approx_equal} 0.25 after the heating power was switched off. Small-scale fluctuations of the electron density were studied with the help of correlation reflectometry. It was found that, in a narrow region near {rho} {approx_equal} 0.25, the amplitude of the density fluctuations was two times lower than that in the ohmic heating phase. Quasi-coherent fluctuations were suppressed over a period of time during which the steep temperature gradient existed. Measurements of the poloidal rotation velocity of turbulent fluctuations show that there is no velocity shear after the heating is switched off. An analysis of the linear growth rates of instabilities shows that the ion-temperature-gradient mode is unstable at {rho} {approx_equal} 0.25 throughout the entire discharge phase. The effect observed can be explained by an increase in the distance between the rational surfaces near the radius at which the safety factor is q = 1 due to the temporary flattening of the q profile after the off-axis electron-cyclotron resonance heating is switched off.

  11. Magnetic resonance spectroscopy in vivo of neurochemicals in a transgenic model of Alzheimer's disease: a longitudinal study of metabolites, relaxation time, and behavioral analysis in TASTPM and wild-type mice.

    PubMed

    Forster, Duncan; Davies, Karen; Williams, Steve

    2013-04-01

    Alzheimer's disease (AD) is the most common form of dementia in the elderly. Due to ongoing advances in our understanding of the underlying pathology of AD, many potential new targets for therapeutics are becoming available. Transgenic mouse models of AD have helped in furthering our understanding of AD and also provide a vehicle for preclinical testing of new, putative disease-modifying therapeutics, which may have potential for translation to use in clinical trials. To identify possible translational biomarkers, we have studied the longitudinal cerebral metabolic pattern of the TASTPM transgenic AD mouse, a double transgenic mouse overexpressing human mutant amyloid precursor protein (hAPP695swe) and presenilin-1 (M146V) by (1) H magnetic resonance spectroscopy, along with concurrent brain T1 /T2 mapping and behavioral testing. We found significant differences in creatine, glutamate, N-acetylaspartate, choline-containing compounds, and myo-inositol between TASTPM and wild-type mice. In the case of N-acetylaspartate and myo-inositol, there were similarities to differences detected in human AD. T1 /T2 values were shorter overall in TASTPM mice, indicating possible differences in water content between TASTPM and wild-type mice. In older TASTPM mice, exploratory behavior became more random, indicating a possible memory deficiency. The decrease in behavioral performance correlated in the transgenic group with higher expression of myo-inositol.

  12. Ferromagnetic critical behavior in U(Co1-xFex)Al (0 ≤x ≤0.02 ) studied by 59Co nuclear quadrupole resonance measurements

    NASA Astrophysics Data System (ADS)

    Karube, K.; Hattori, T.; Ishida, K.; Kimura, N.

    2015-02-01

    In order to investigate physical properties around a ferromagnetic (FM) quantum transition point and a tricritical point (TCP) in the itinerant-electron metamagnetic compound UCoAl, we have performed the 59Co nuclear quadrupole resonance (NQR) measurement for the Fe-substituted U(Co1-xFex)Al(x =0 ,0.5 ,1 ,and2 %) in zero external magnetic field. The Fe concentration dependence of 59Co -NQR spectra at low temperatures indicates that the first-order FM transition occurs at least above x =1 % . The magnetic fluctuations along the c axis detected by the nuclear spin-spin relaxation rate 1 /T2 exhibit an anomaly at Tmax˜20 K and enhance with increasing x . These results are in good agreement with theoretical predictions and indicate the presence of prominent critical fluctuations at the TCP in this system.

  13. Synthesis, characterization, and photophysical properties of Bodipy-spirooxazine and -spiropyran conjugates: modulation of fluorescence resonance energy transfer behavior via acidochromic and photochromic switching.

    PubMed

    Kong, Lingcan; Wong, Hok-Lai; Tam, Anthony Yiu-Yan; Lam, Wai Han; Wu, Lixin; Yam, Vivian Wing-Wah

    2014-02-12

    Two series of Bodipy-containing photochromic spirooxazine and spiropyran derivatives have been designed, synthesized and characterized by (1)H NMR, ESI mass spectrometry and elemental analysis. Their electrochemical and photochromic properties were investigated. The photophysical, ultrafast transient absorption, and fluorescence resonance energy transfer (FRET) properties from Bodipy (donor) to the ring-opened merocyanine (acceptor) were also studied. Upon photoexcitation, all the photochromic spirooxazine- and spiropyran-containing compounds exhibited reversible photochromism. Computational studies have been performed to provide further insights into the nature of the electronic transitions for the two classes of compounds. The rate constants and activation parameters for thermal bleaching reactions of compounds SO, SP-alkyne, 1-3, and 8-10 were determined through kinetic studies in acetonitrile. The thermal bleaching reaction rate of the spiropyran-containing compounds is found to be much slower than that of the spirooxazine-containing counterparts.

  14. Resonance Trapping in Planetary Systems

    NASA Astrophysics Data System (ADS)

    Pour, Nader H.

    1998-09-01

    We study dynamics of a planetary system that consists of a star and two planets taking into account dynamical friction. Numerical integrations of a restricted planar circular three body model of this system indicate resonance capture. The main purpose of this paper is to present the results of an extensive numerical experiment performed on this model and also to present analytical arguments for the observed resonance trapping and its consequences. The equations of motion are written in terms of Delaunay variables and the recently developed method of partial averaging near resonance* is employed in order to account for the behavior of the system at resonance. * C.Chicone, B.Mashhoon and D.Retzloff, Ann.Inst.Henri Poincare, Vol.64, no 1, 1996, p.87-125.

  15. Tunable Micro- and Nanomechanical Resonators

    PubMed Central

    Zhang, Wen-Ming; Hu, Kai-Ming; Peng, Zhi-Ke; Meng, Guang

    2015-01-01

    Advances in micro- and nanofabrication technologies have enabled the development of novel micro- and nanomechanical resonators which have attracted significant attention due to their fascinating physical properties and growing potential applications. In this review, we have presented a brief overview of the resonance behavior and frequency tuning principles by varying either the mass or the stiffness of resonators. The progress in micro- and nanomechanical resonators using the tuning electrode, tuning fork, and suspended channel structures and made of graphene have been reviewed. We have also highlighted some major influencing factors such as large-amplitude effect, surface effect and fluid effect on the performances of resonators. More specifically, we have addressed the effects of axial stress/strain, residual surface stress and adsorption-induced surface stress on the sensing and detection applications and discussed the current challenges. We have significantly focused on the active and passive frequency tuning methods and techniques for micro- and nanomechanical resonator applications. On one hand, we have comprehensively evaluated the advantages and disadvantages of each strategy, including active methods such as electrothermal, electrostatic, piezoelectrical, dielectric, magnetomotive, photothermal, mode-coupling as well as tension-based tuning mechanisms, and passive techniques such as post-fabrication and post-packaging tuning processes. On the other hand, the tuning capability and challenges to integrate reliable and customizable frequency tuning methods have been addressed. We have additionally concluded with a discussion of important future directions for further tunable micro- and nanomechanical resonators. PMID:26501294

  16. Functional Magnetic Resonance Imaging and Pediatric Anxiety

    ERIC Educational Resources Information Center

    Pine, Daniel S.; Guyer, Amanda E.; Leibenluft, Ellen; Peterson, Bradley S.; Gerber, Andrew

    2008-01-01

    The use of functional magnetic resonance imaging in investigating pediatric anxiety disorders is studied. Functional magnetic resonance imaging can be utilized in demonstrating parallels between the neural architecture of difference in anxiety of humans and the neural architecture of attention-orienting behavior in nonhuman primates or rodents.…

  17. Meson resonances on the lattice

    SciTech Connect

    Edwards, Robert G.

    2016-06-01

    There has been recent, significant, advances in the determination of the meson spectrum of QCD. Current efforts have focused on the development and application of finite-volume formalisms that allow for the determination of scattering amplitudes as well as resonance behavior in coupled channel systems. I will review some of these recent developments, and demonstrate the viability of the method in meson systems

  18. Meson Resonances from Lattice QCD

    SciTech Connect

    Edwards, Robert G.

    2016-06-01

    There has been recent, significant, advances in the determination of the meson spectrum of QCD. Current efforts have focused on the development and application of finite-volume formalisms that allow for the determination of scattering amplitudes as well as resonance behavior in coupled channel systems. I will review some of these recent developments, and demonstrate the viability of the method in meson systems.

  19. Sandwich-like Cu(1.94)S-ZnS-Cu(1.94)S nanoheterostructure: structure, formation mechanism and localized surface plasmon resonance behavior.

    PubMed

    Huang, Feng; Xu, Ju; Chen, Daqin; Wang, Yuansheng

    2012-10-26

    In this communication, a thermolysis route is developed to synthesize novel Cu(1.94)S-ZnS-Cu(1.94)S nanoheterostructures with interesting sandwich-like architectures, taking Cu(1.94)S nanoplates as precursors. Evidently, the trimeric nanostructure is formed by a three-stage process, which includes the Zn-oleate induced assembling of Cu(1.94)S nanoplate couples, the heteronucleation and growth of a ZnS layer between two Cu(1.94)S plates dominated by interfacial diffusion, and the catalyst assisted axial growth of ZnS nanorod following the solution-liquid-solid mechanism. With epitaxial growth of ZnS nanocrystal between two Cu(1.94)S nanoplates, the localized surface plasmon resonance frequency of Cu(1.94)S shifts from 1875 to 1323 nm, indicating that this new material is potentially applicable as a light absorbing agent in laser photothermal therapy. The reported growth mechanism may provide new strategies for designing and fabricating various technologically important polymeric nanoheterostructures.

  20. Light-dependent and -independent behavioral effects of extremely low frequency magnetic fields in a land snail are consistent with a parametric resonance mechanism

    SciTech Connect

    Prato, F.S.; Thomas, A.W. |; Kavaliers, M.; Cullen, A.P.

    1997-05-01

    Exposure to extremely low frequency (ELF) magnetic fields has been shown to attenuate endogenous opioid peptide mediated antinociception or analgesia in the terrestrial pulmonate snail, Cepaea nemoralis. Here the authors examine the roles of light in determining this effect and address the mechanisms associated with mediating the effects of the ELF magnetic fields in both the presence and absence of light. Specifically, they consider whether the magnetic field effects involve an indirect induced electric current mechanism or a direct effect such as a parametric resonance mechanism (PRM). They exposed snails in both the presence and absence of light at three different frequencies (30, 60, and 120 Hz) with static field values (B{sub DC}) and ELF magnetic field amplitude (peak) and direction (B{sub AC}) set according to the predictions of the PRM for Ca{sup 2+}. Analgesia was induced in snails by injecting them with an enkephalinase inhibitor, which augments endogenous opioid (enkephalin) activity. They found that the magnetic field exposure reduced this opioid-induced analgesia significantly more if the exposure occurred in the presence rather than the absence of light. However, the percentage reduction in analgesia in both the presence and absence of light was not dependent on the ELF frequency. This finding suggests that in both the presence and the absence of light the effect of the ELF magnetic field was mediated by a direct magnetic field detection mechanism such as the PRM rather than an induced current mechanism.

  1. Study of the magnetic properties of the Cex La1-x Pt alloy system: Which interaction establishes ferromagnetism in Kondo systems?

    NASA Astrophysics Data System (ADS)

    Očko, M.; Zadro, K.; Drobac, Đ.; Aviani, I.; Salamon, K.; Mixson, D.; Bauer, E. D.; Sarrao, J. L.

    2016-11-01

    In order to study Kondo ferromagnetism, particularly of the CePt compound, we investigate the magnetic properties of the CexLa1-xPt alloy system in the temperature range from 1.8 K to 320 K. The results of these investigations can be summarized as follows: dc-susceptibility can be described by the Curie-Weiss law at higher temperatures down to about 100 K, but also at the low temperatures above the phase transition. At higher temperatures, the extracted Curie-Weiss constant, θp, is negative in contrast to the low temperatures, where θC is positive. The extracted effective magnetic moment from the higher temperatures is the same for all the alloys and is close to the theoretical value of the isolated Ce3+ ion, μ=2.54 μB, indicating the hybridization is weak and, and consequently, Kondo interaction is weak. These observations confirm the main important conclusions inferred from an earlier transport properties investigation of this alloy system. The Curie temperature extracted by various approaches was compared to the extraction from the ac-susceptibility measurements. We show that its concentration dependence is not consistent with Doniach's diagram. Hence, RKKY interaction is not responsible for the ferromagnetism in this alloy system.

  2. Doping Effects on the Electronic Structure of an Anisotropic Kondo Semiconductor CeOs2Al10: An Optical Study with Re and Ir Substitution

    NASA Astrophysics Data System (ADS)

    Kimura, Shin-ichi; Takao, Hitoshi; Kawabata, Jo; Yamada, Yoshihiro; Takabatake, Toshiro

    2016-12-01

    An anisotropic Kondo semiconductor CeOs2Al10 exhibits an unusual antiferromagnetic order at rather high transition temperature T0 of 28.5 K. Two possible origins of the magnetic order have been proposed so far, one is the Kondo coupling of the hybridization between the conduction (c) and the 4f states and the other is the charge-density wave/charge ordering along the orthorhombic b-axis. To clarify the origin of the magnetic order, we have investigated the electronic structure of hole- and electron-doped CeOs2Al10 [Ce(Os1-yRey)2Al10 and Ce(Os1-xIrx)2Al10, respectively] by using optical conductivity spectra along the b-axis. The intensity of the c-f hybridization gap at ħω ˜ 50 meV continuously decreases from y = 0.10 to x = 0.12 via x = y = 0. On the other hand, the intensity of the charge excitation observed at ħω ˜ 20 meV has the maximum at x = y = 0 as similar with the doping dependence of T0. The fact that the charge excitation is strongly related to the magnetic order strengthens the possibility of the charge density wave/charge ordering as the origin of the magnetic order.

  3. Upper critical field and Kondo effects in Fe(Te0.9Se0.1) thin films by pulsed field measurements

    SciTech Connect

    Salamon, Myron B.; Cornell, Nicholas; Jaime, Marcelo; Balakirev, Fedor F.; Zakhidov, Anvar; Huang, Jijie; Wang, Haiyan

    2016-02-10

    The transition temperatures of epitaxial films of Fe(Te0:9Se0:1) are remarkably insensitive to applied magnetic field, leading to predictions of upper critical fields Bc2(T = 0) in excess of 100 T. Using pulsed magnetic fields, we find Bc2(0) to be on the order of 45 T, similar to values in bulk material and still in excess of the paramagnetic limit. The same films show strong magnetoresistance in fields above Bc2(T), consistent with the observed Kondo minimum seen above Tc. Fits to the temperature dependence in the context of the WHH model, using the experimental value of the Maki parameter, require an effective spin-orbit relaxation parameter of order unity. Lastly, we suggest that Kondo localization plays a similar role to spin-orbit pair breaking in making WHH fits to the data.

  4. Polynomial expansion Monte Carlo study of frustrated itinerant electron systems: Application to a spin-ice type Kondo lattice model on a pyrochlore lattice

    NASA Astrophysics Data System (ADS)

    Ishizuka, Hiroaki; Udagawa, Masafumi; Motome, Yukitoshi

    2013-12-01

    We present the benchmark of the polynomial expansion Monte Carlo method to a Kondo lattice model with classical localized spins on a geometrically frustrated lattice. The method enables us to reduce the calculation amount by using the Chebyshev polynomial expansion of the density of states compared to a conventional Monte Carlo technique based on the exact diagonalization of the fermion Hamiltonian matrix. Further reduction is brought about by a real-space truncation of the vector-matrix operations. We apply the method to the model with spin-ice type Ising spins on a three-dimensional pyrochlore lattice and carefully examine the convergence in terms of the order of polynomials and the truncation distance. We find that, in a wide range of electron density at a relatively weak Kondo coupling compared to the noninteracting bandwidth, the results by the polynomial expansion method show good convergence to those by the conventional method within reasonable numbers of polynomials. This enables us to study the systems up to 4×83=2048 sites, while the previous study by the conventional method was limited to 4×43=256 sites. On the other hand, the real-space truncation is not helpful in reducing the calculation amount for the system sizes that we reached, as the sufficient convergence is obtained when most of the sites are involved within the truncation distance. The necessary truncation distance, however, appears not to show significant system size dependence, suggesting that the truncation method becomes efficient for larger system sizes.

  5. Photonic band structure and effective medium properties of doubly-resonant core-shell metallo-dielectric nanowire arrays: low-loss, isotropic optical negative-index behavior

    NASA Astrophysics Data System (ADS)

    Abujetas, D. R.; Paniagua-Domínguez, R.; Nieto-Vesperinas, M.; Sánchez-Gil, J. A.

    2015-12-01

    We investigate theoretically and numerically the photonic band structure in the optical domain of an array of core-shell metal-semiconductor nanowires. Corresponding negative-index photonic bands are calculated, showing isotropic equifrequency surfaces. The effective (negative) electric permittivity and magnetic permeability, retrieved from S-parameters, are used to compare the performance of such nanowire arrays with homogeneous media in canonical examples, such as refraction through a prism and flat-lens focusing. Very good agreement is found, confirming the effective medium behavior of the nanowire array as a low-loss, isotropic (2D) and bulk, optical negative index metamaterial. Indeed, disorder is introduced to further stress its robustness.

  6. The genetic diversity,relationships,and potential for biological control of the lobate lac scale,Paratachardina pseudolobata Kondo&Gullan(Hemiptera:Coccoidea:Kerriidae),a pest in Florida,the Bahamas,Cuba and Christmas Island

    Technology Transfer Automated Retrieval System (TEKTRAN)

    The lobate lac scale Paratachardina pseudolobata Kondo & Gullan (Kerriidae) is a polyphagous pest of woody plants in Florida (U.S.A), the Bahamas, Cuba, and Christmas Island (Australia). Its recent appearance as a pest in these places indicates that this scale is introduced; however, its native rang...

  7. Stochastic resonance in nanomechanical systems

    NASA Astrophysics Data System (ADS)

    Badzey, Robert L.

    The phenomenon of stochastic resonance is a counter-intuitive one: adding noise to a noisy nonlinear system under the influence of a modulation results in coherent behavior. The signature of the effect is a resonance in the signal-to-noise ratio of the response over a certain range of noise power; this behavior is absent if either the modulation or the noise are absent. Stochastic resonance has attracted considerable interest over the past several decades, having been seen in a great number of physical and biological systems. Here, observation of stochastic resonance is reported for nanomechanical systems consisting of a doubly-clamped beam resonators fabricated from single-crystal silicon. Such oscillators have been found to display nonlinear and bistable behavior under the influence of large driving forces. This bistability is exploited to produce a controllable nanomechanical switch, a device that may be used as the basis for a new generation of computational memory elements. These oscillators possess large intrinsic resonance frequencies (MHz range or higher) due to their small size and relatively high stiffness; thus they have the potential to rival the current state-of-the-art of electronic and magnetic storage technologies. This small size also allows them to be packed in densities which meet or exceed the superparamagnetic limit for magnetic storage media of 100 GB/in2. Two different doubly-clamped beams were cooled to low temperatures (300 mK--4 K), and excited with a magnetomotive technique. They were driven into the nonlinear response regime, and then modulated to induce switching between their bistable states. When the modulation was reduced, the switching died out. Application of noise, either with an external broadband source or via an increase in temperature, resulted in a distinct resonance in the signal-to-noise ratio. Aside from establishing the phenomenon of stochastic resonance in yet another physical system, the observation of this effect has

  8. Secondary resonances of electrically actuated resonant microsensors

    NASA Astrophysics Data System (ADS)

    Abdel-Rahman, Eihab M.; Nayfeh, Ali H.

    2003-05-01

    We investigate the response of a microbeam-based resonant sensor to superharmonic and subharmonic electric actuations using a model that incorporates the nonlinearities associated with moderately large displacements and electric forces. The method of multiple scales is used, in each case, to obtain two first-order nonlinear ordinary-differential equations that describe the modulation of the amplitude and phase of the response and its stability. We present typical frequency-response and force-response curves demonstrating, in both cases, the coexistence of multivalued solutions. The solution corresponding to a superharmonic excitation consists of three branches, which meet at two saddle-node bifurcation points. The solution corresponding to a subharmonic excitation consists of two branches meeting a branch of trivial solutions at two pitchfork bifurcation points. One of these bifurcation points is supercritical and the other is subcritical. The results provide an analytical tool to predict the microsensor response to superharmonic and subharmonic excitations, specifically the locations of sudden jumps and regions of hysteretic behavior, thereby enabling designers to safely use these frequencies as measurement signals. They also allow designers to examine the impact of various design parameters on the device behavior.

  9. Neutron diffraction study of magnetic field induced behavior in the heavy Fermion Ce3Co4Sn13

    SciTech Connect

    Christianson, Andrew D; Goremychkin, E. A.; Gardner, J. S.; Kang, H. J.; Chung, J.-H.; Manuel, P.; Thompson, J. D.; Sarrao, J. L.; Lawrence, J. M.

    2008-01-01

    The specific heat of Ce3Co4Sn13 exhibits a crossover from heavy Fermion behavior with antiferromagnetic correlations at low field to single impurity Kondo behavior above 2 T. We have performed neutron diffraction measurements in magnetic fields up to 6 Tesla on single crystal samples. The (001) position shows a dramatic increase in intensity in field which appears to arise from static polarization of the 4f level and which at 0.14 K also exhibits an anomaly near 2T reflecting the crossover to single impurity behavior.

  10. A Comparison of Magnetic Resonance Imaging and Neuropsychological Examination in the Diagnostic Distinction of Alzheimer's Disease and Behavioral Variant Frontotemporal Dementia

    PubMed Central

    Wang, Jingjing; Redmond, Stephen J.; Bertoux, Maxime; Hodges, John R.; Hornberger, Michael

    2016-01-01

    The clinical distinction between Alzheimer's disease (AD) and behavioral variant frontotemporal dementia (bvFTD) remains challenging and largely dependent on the experience of the clinician. This study investigates whether objective machine learning algorithms using supportive neuroimaging and neuropsychological clinical features can aid the distinction between both diseases. Retrospective neuroimaging and neuropsychological data of 166 participants (54 AD; 55 bvFTD; 57 healthy controls) was analyzed via a Naïve Bayes classification model. A subgroup of patients (n = 22) had pathologically-confirmed diagnoses. Results show that a combination of gray matter atrophy and neuropsychological features allowed a correct classification of 61.47% of cases at clinical presentation. More importantly, there was a clear dissociation between imaging and neuropsychological features, with the latter having the greater diagnostic accuracy (respectively 51.38 vs. 62.39%). These findings indicate that, at presentation, machine learning classification of bvFTD and AD is mostly based on cognitive and not imaging features. This clearly highlights the urgent need to develop better biomarkers for both diseases, but also emphasizes the value of machine learning in determining the predictive diagnostic features in neurodegeneration. PMID:27378905

  11. Experiments with Helmholtz Resonators.

    ERIC Educational Resources Information Center

    Greenslade, Thomas B., Jr.

    1996-01-01

    Presents experiments that use Helmholtz resonators and have been designed for a sophomore-level course in oscillations and waves. Discusses the theory of the Helmholtz resonator and resonance curves. (JRH)

  12. MRI (Magnetic Resonance Imaging)

    MedlinePlus

    ... and Procedures Medical Imaging MRI (Magnetic Resonance Imaging) MRI (Magnetic Resonance Imaging) Share Tweet Linkedin Pin it More sharing options ... usually given through an IV in the arm. MRI Research Programs at FDA Magnetic Resonance Imaging (MRI) ...

  13. Thermally tunable slot-coupled dielectric resonator antenna

    NASA Astrophysics Data System (ADS)

    Bi, Ke; Chen, Cong; Wang, Qingmin; Liu, Wenjun; Hao, Yanan; Gao, Xinlu; Huang, Shanguo; Lei, Ming

    2017-02-01

    A thermally tunable slot-coupled dielectric resonator antenna (DRA) has been designed and prepared by placing a thermosensitive ceramic resonator onto the slot. Typical magnetic resonance occurs in the resonator, which is closely related to its dielectric constant. Because the dielectric constant of the ceramic resonator decreases as the temperature increases, the resonance frequency of the proposed DRA increases as the temperature increases. The simulated results are in good agreement with the measured ones, which confirms the thermally tunable behavior. This approach provides a way for designing the frequency tunable antennas.

  14. Regenerative feedback resonant circuit

    DOEpatents

    Jones, A. Mark; Kelly, James F.; McCloy, John S.; McMakin, Douglas L.

    2014-09-02

    A regenerative feedback resonant circuit for measuring a transient response in a loop is disclosed. The circuit includes an amplifier for generating a signal in the loop. The circuit further includes a resonator having a resonant cavity and a material located within the cavity. The signal sent into the resonator produces a resonant frequency. A variation of the resonant frequency due to perturbations in electromagnetic properties of the material is measured.

  15. Development and Reproduction of Brethesiella cf. abnormicornis (Girault) (Hymenoptera: Encyrtidae), a Parasitoid of the Colombian Fluted Scale, Crypticerya multicicatrices Kondo & Unruh (Hemiptera: Monophlebidae).

    PubMed

    Montealegre, X; Sotelo, P; Kondo, T

    2016-04-01

    Studies on the development and reproduction of Brethesiella cf. abnormicornis (Girault) (Hymenoptera: Encyrtidae), a parasitoid of the Colombian fluted scale, Crypticerya multicicatrices Kondo & Unruh (Hemiptera: Monophlebidae), were conducted under laboratory conditions. The duration of the life cycle, adult longevity, fecundity, and population parameters were determined. The parasitoid takes about 29 d to complete a single generation (from egg to adult). In addition, population parameters show that one female wasp is replaced by nearly 32 females, with a female-to-male sex ratio of 2:1. Population parameters estimated in this study can be considered baseline information for a mass-rearing protocol. This is the first detailed study of the biology of a species of Brethesiella, where the duration of all larval stages of the parasitoid is determined, being an important contribution for further biological studies of endoparasitoids.

  16. Magnetic structure of the antiferromagnetic Kondo lattice compounds CeRhAl4Si2 and CeIrAl4Si2

    DOE PAGES

    Ghimire, N. J.; Calder, S.; Janoschek, M.; ...

    2015-06-01

    In this article, we have investigated the magnetic ground state of the antiferromagnetic Kondo-lattice compounds CeMAl4Si2(M = Rh, Ir) using neutron powder diffraction. Although both of these compounds show two magnetic transitions TN1 and TN2 in the bulk properties measurements, evidence for magnetic long-range order was only found below the lower transition TN2. Analysis of the diffraction profiles reveals a commensurate antiferromagnetic structure with a propagation vector k = (0, 0, 1/2). The magnetic moment in the ordered state of CeRhAl4Si2 and CeIrAl4Si2 were determined to be 1.14(2) and 1.41(3) μB/Ce, respectively, and are parallel to the crystallographic c-axis inmore » agreement with magnetic susceptibility measurements.« less

  17. Triad mode resonant interactions in suspended cables

    NASA Astrophysics Data System (ADS)

    Guo, TieDing; Kang, HouJun; Wang, LianHua; Zhao, YueYu

    2016-03-01

    A triad mode resonance, or three-wave resonance, is typical of dynamical systems with quadratic nonlinearities. Suspended cables are found to be rich in triad mode resonant dynamics. In this paper, modulation equations for cable's triad resonance are formulated by the multiple scale method. Dynamic conservative quantities, i.e., mode energy and Manley-Rowe relations, are then constructed. Equilibrium/dynamic solutions of the modulation equations are obtained, and full investigations into their stability and bifurcation characteristics are presented. Various bifurcation behaviors are detected in cable's triad resonant responses, such as saddle-node, Hopf, pitchfork and period-doubling bifurcations. Nonlinear behaviors, like jump and saturation phenomena, are also found in cable's responses. Based upon the bifurcation analysis, two interesting properties associated with activation of cable's triad resonance are also proposed, i.e., energy barrier and directional dependence. The first gives the critical amplitude of high-frequency mode to activate cable's triad resonance, and the second characterizes the degree of difficulty for activating cable's triad resonance in two opposite directions, i.e., with positive or negative internal detuning parameter.

  18. Electroexcitation of nucleon resonances

    SciTech Connect

    Inna Aznauryan, Volker D. Burkert

    2012-01-01

    We review recent progress in the investigation of the electroexcitation of nucleon resonances, both in experiment and in theory. The most accurate results have been obtained for the electroexcitation amplitudes of the four lowest excited states, which have been measured in a range of Q2 up to 8 and 4.5 GeV2 for the Delta(1232)P33, N(1535)S11 and N(1440)P11, N(1520)D13, respectively. These results have been confronted with calculations based on lattice QCD, large-Nc relations, perturbative QCD (pQCD), and QCD-inspired models. The amplitudes for the Delta(1232) indicate large pion-cloud contributions at low Q2 and don't show any sign of approaching the pQCD regime for Q2<7 GeV2. Measured for the first time, the electroexcitation amplitudes of the Roper resonance, N(1440)P11, provide strong evidence for this state as a predominantly radial excitation of a three-quark (3q) ground state, with additional non-3-quark contributions needed to describe the low Q2 behavior of the amplitudes. The longitudinal transition amplitude for the N(1535)S11 was determined and has become a challenge for quark models. Explanations may require large meson-cloud contributions or alternative representations of this state. The N(1520)D13 clearly shows the rapid changeover from helicity-3/2 dominance at the real photon point to helicity-1/2 dominance at Q2 > 0.5 GeV2, confirming a long-standing prediction of the constituent quark model. The interpretation of the moments of resonance transition form factors in terms of transition transverse charge distributions in infinite momentum frame is presented.

  19. Resonance beyond frequency-matching: multidimensional resonance

    NASA Astrophysics Data System (ADS)

    Wang, Zhenyu; Li, Mingzhe; Wang, Ruifang

    2017-03-01

    Resonance, conventionally defined as the oscillation of a system when the temporal frequency of an external stimulus matches a natural frequency of the system, is important in both fundamental physics and applied disciplines. However, the spatial character of oscillation is not considered in this definition. We reveal the creation of spatial resonance when the stimulus matches the space pattern of a normal mode in an oscillating system. The complete resonance, which we call multidimensional resonance, should be a combination of both the temporal and the spatial resonance. We further elucidate that the spin wave produced by multidimensional resonance drives considerably faster reversal of the vortex core in a magnetic nanodisc. Multidimensional resonance provides insight into the nature of wave dynamics and opens the door to novel applications.

  20. Nucleon Resonance Transition Form factors

    SciTech Connect

    Burkert, Volker D.; Mokeev, Viktor I.; Aznauryan, Inna G.

    2016-08-01

    We discuss recent results from CLAS on electromagnetic resonance transition amplitudes and their dependence on the distance scale (Q2). From the comparison of these results with most advanced theoretical calculations within QCD-based approaches there is clear evidence that meson-baryon contributions are present and important at large distances, i.e. small Q2, and that quark core contributions dominate the short distance behavior.

  1. Scaling the Kondo lattice.

    PubMed

    Yang, Yi-feng; Fisk, Zachary; Lee, Han-Oh; Thompson, J D; Pines, David

    2008-07-31

    The origin of magnetic order in metals has two extremes: an instability in a liquid of local magnetic moments interacting through conduction electrons, and a spin-density wave instability in a Fermi liquid of itinerant electrons. This dichotomy between 'local-moment' magnetism and 'itinerant-electron' magnetism is reminiscent of the valence bond/molecular orbital dichotomy present in studies of chemical bonding. The class of heavy-electron intermetallic compounds of cerium, ytterbium and various 5f elements bridges the extremes, with itinerant-electron magnetic characteristics at low temperatures that grow out of a high-temperature local-moment state. Describing this transition quantitatively has proved difficult, and one of the main unsolved problems is finding what determines the temperature scale for the evolution of this behaviour. Here we present a simple, semi-quantitative solution to this problem that provides a basic framework for interpreting the physics of heavy-electron materials and offers the prospect of a quantitative determination of the physical origin of their magnetic ordering and superconductivity. It also reveals the difference between the temperature scales that distinguish the conduction electrons' response to a single magnetic impurity and their response to a lattice of local moments, and provides an updated version of the well-known Doniach diagram.

  2. Cavity- and waveguide-resonators in electron paramagnetic resonance, nuclear magnetic resonance, and magnetic resonance imaging.

    PubMed

    Webb, Andrew

    2014-11-01

    Cavity resonators are widely used in electron paramagnetic resonance, very high field magnetic resonance microimaging and also in high field human imaging. The basic principles and designs of different forms of cavity resonators including rectangular, cylindrical, re-entrant, cavity magnetrons, toroidal cavities and dielectric resonators are reviewed. Applications in EPR and MRI are summarized, and finally the topic of traveling wave MRI using the magnet bore as a waveguide is discussed.

  3. Static and Dynamic Behavior of Quartz Resonators

    DTIC Science & Technology

    1979-07-01

    representative of a long line of 110] W. J. Spencer and W. L. Smith , "Precision crystal frequency stan- dards," in Poc. 15th AFC3, May-June 1961, pp...1963, pp. 248- 266. The actual frequency instabilities observed in quartz crystal 1121 W. L. Smith and W. J. Spencer, "Quartz crystal thermometer for...for improved appear in Proc. 33rd AFCS, May-June 1979. quartz crystal oscillator performance," IEEE Trans. Instrum. [411 G. Theobald , G. Marianneau, R

  4. Resistive cooling circuits for charged particle traps using crystal resonators.

    PubMed

    Kaltenbacher, T; Caspers, F; Doser, M; Kellerbauer, A; Pribyl, W

    2011-11-01

    The paper addresses a novel method to couple a signal from charged particles in a Penning trap to a high Q resonant circuit using a crystal resonator. Traditionally, the trap capacity is converted into a resonator by means of an inductance. The tuned circuit's Q factor is directly linked to the input impedance "seen" by the trapped particles at resonance frequency. This parallel resonance impedance is a measure of the efficiency of resistive cooling and thus it should be optimized. We propose here a commercially available crystal resonator since it exhibits a very high Q value and a parallel resonance impedance of several MΩ. The possibility to tune the parallel resonance frequency of the quartz results in filter behavior that allows covering a range of some tens of its 3dB bandwidth by means of tuning.

  5. Integral resonator gyroscope

    NASA Technical Reports Server (NTRS)

    Shcheglov, Kirill V. (Inventor); Challoner, A. Dorian (Inventor); Hayworth, Ken J. (Inventor); Wiberg, Dean V. (Inventor); Yee, Karl Y. (Inventor)

    2008-01-01

    The present invention discloses an inertial sensor having an integral resonator. A typical sensor comprises a planar mechanical resonator for sensing motion of the inertial sensor and a case for housing the resonator. The resonator and a wall of the case are defined through an etching process. A typical method of producing the resonator includes etching a baseplate, bonding a wafer to the etched baseplate, through etching the wafer to form a planar mechanical resonator and the wall of the case and bonding an end cap wafer to the wall to complete the case.

  6. Asteroid Secular Resonant Proper Elements

    NASA Astrophysics Data System (ADS)

    Morbidelli, Alessandro

    1993-09-01

    A practical algorithm for the computation of the dynamic evolution of asteroids which are inside or close to a secular resonance has been developed. The results are checked with many numerical simulations of both real and fictitious objects. These tests prove that the algorithm is able to identify the dynamic nature of resonant objects and distinguish between future planet crossers and regular bodies. The short CPU time necessary for its execution makes it a useful tool for studying the mechanisms of meteorite transport to the inner Solar System. For this purpose, the sets of initial conditions which lead to large eccentricity in the v6 secular resonance are identified. Finally, the dynamic behavior of 44 numbered asteroids very close to the v6 resonance is analyzed. Only 4 of these asteroids are found in regions dangerous for their stability. A few others become temporary Mars crossers. The rest of them, as 6 Hebe, have a moderate eccentricity during all their quasi-periodic dynamic evolution.

  7. Controlling metamaterial resonances with light

    SciTech Connect

    Chakrabarti, Sangeeta; Ramakrishna, S. Anantha; Wanare, Harshawardhan

    2010-08-15

    We investigate the use of coherent optical fields as a means of dynamically controlling the resonant behavior of a variety of composite metamaterials, wherein the metamaterial structures are embedded in a dispersive dielectric medium. Control and switching are implemented by coherently driving the resonant permittivity of the embedding medium with applied optical radiation. The effect of embedding split ring resonators in a frequency-dispersive medium with Lorentz-like dispersion or with dispersion engineered by electromagnetically induced transparency (EIT) is manifested in the splitting of the negative-permeability band, the modified (frequency-dependent) filling fractions, and the dissipation factors. The modified material parameters are strongly linked to the resonant frequencies of the medium, and for an embedding medium exhibiting EIT also to the strength and detuning of the control field. The robustness of control against the deleterious influence of dissipation associated with the metallic structures as well as the inhomogeneous broadening due to structural imperfections is demonstrated. Studies on plasmonic metamaterials that consist of metallic nanorods arranged in loops and exhibit a collective magnetic response at optical frequencies are presented. Control and switching in this class of plasmonic nanorod metamaterials is shown to be possible, for example, by embedding these arrays in a Raman-active liquid like CS{sub 2} and utilizing the inverse Raman effect.

  8. Partially orthogonal resonators for magnetic resonance imaging

    PubMed Central

    Chacon-Caldera, Jorge; Malzacher, Matthias; Schad, Lothar R.

    2017-01-01

    Resonators for signal reception in magnetic resonance are traditionally planar to restrict coil material and avoid coil losses. Here, we present a novel concept to model resonators partially in a plane with maximum sensitivity to the magnetic resonance signal and partially in an orthogonal plane with reduced signal sensitivity. Thus, properties of individual elements in coil arrays can be modified to optimize physical planar space and increase the sensitivity of the overall array. A particular case of the concept is implemented to decrease H-field destructive interferences in planar concentric in-phase arrays. An increase in signal to noise ratio of approximately 20% was achieved with two resonators placed over approximately the same planar area compared to common approaches at a target depth of 10 cm at 3 Tesla. Improved parallel imaging performance of this configuration is also demonstrated. The concept can be further used to increase coil density. PMID:28186135

  9. Partially orthogonal resonators for magnetic resonance imaging

    NASA Astrophysics Data System (ADS)

    Chacon-Caldera, Jorge; Malzacher, Matthias; Schad, Lothar R.

    2017-02-01

    Resonators for signal reception in magnetic resonance are traditionally planar to restrict coil material and avoid coil losses. Here, we present a novel concept to model resonators partially in a plane with maximum sensitivity to the magnetic resonance signal and partially in an orthogonal plane with reduced signal sensitivity. Thus, properties of individual elements in coil arrays can be modified to optimize physical planar space and increase the sensitivity of the overall array. A particular case of the concept is implemented to decrease H-field destructive interferences in planar concentric in-phase arrays. An increase in signal to noise ratio of approximately 20% was achieved with two resonators placed over approximately the same planar area compared to common approaches at a target depth of 10 cm at 3 Tesla. Improved parallel imaging performance of this configuration is also demonstrated. The concept can be further used to increase coil density.

  10. Neutron resonance averaging

    SciTech Connect

    Chrien, R.E.

    1986-10-01

    The principles of resonance averaging as applied to neutron capture reactions are described. Several illustrations of resonance averaging to problems of nuclear structure and the distribution of radiative strength in nuclei are provided. 30 refs., 12 figs.

  11. Nanomechanical resonance detector

    DOEpatents

    Grossman, Jeffrey C; Zettl, Alexander K

    2013-10-29

    An embodiment of a nanomechanical frequency detector includes a support structure and a plurality of elongated nanostructures coupled to the support structure. Each of the elongated nanostructures has a particular resonant frequency. The plurality of elongated nanostructures has a range of resonant frequencies. An embodiment of a method of identifying an object includes introducing the object to the nanomechanical resonance detector. A resonant response by at least one of the elongated nanostructures of the nanomechanical resonance detector indicates a vibrational mode of the object. An embodiment of a method of identifying a molecular species of the present invention includes introducing the molecular species to the nanomechanical resonance detector. A resonant response by at least one of the elongated nanostructures of the nanomechanical resonance detector indicates a vibrational mode of the molecular species.

  12. Fano resonances in kagome fibers

    NASA Astrophysics Data System (ADS)

    Vincetti, L.; Setti, V.; Zoboli, M.

    2012-06-01

    Confinement Loss of microstructured fibers whose cladding is composed by a triangular arrangement of tubes of various shapes is theoretically and numerically investigated. Kagome Fibers belong from this family of fibers with cladding tubes with hexagonal shape. The shape of the cladding tubes is proved to strongly affect the performance of the microstructured fiber. In order to understand the reasons for this behavior, the spectral properties of the tubes that constitute the cladding are investigated first. It is proved that also these tubes suffer from additional Fano Resonances when they are given a polygonal shape. It is proved that, by using the analytical model developed for the stand alone polygonal tubes, it is possible to predict the spectral position of Fano Resonances also in microstructured fibers. This is extremely important since it suggest new ways to reduce confinement loss in kagome fibers and microstructured fibers in general.

  13. The Electric Giant Resonances

    NASA Astrophysics Data System (ADS)

    van der Woude, A.

    The following sections are included: * Introduction * Experimental Methods to Study Giant Resonances * Introduction * The Tools * Introduction * Tools for Isoscalar Scattering * INELASTIC α-SCATTERING * INELASTIC PROTON SCATTERING * Tools for Isovector Excitations * γ-ABSORPTION AND PARTICLE CAPTURE REACTIONS * CHARGE EXCHANGE REACTIONS - THE (π+, π0) REACTION * Tools For Isoscalar And Isovector Excitations * INELASTIC ELECTRON SCATTERING * GIANT RESONANCE EXCITATION BY FAST HEAVY IONS * From Multipole Cross Section To Multipole Strength * The Electric Isoscalar Resonances * The Isoscalar Giant Monopole Resonance * Systematics on the GMR * Compressibility and the Giant Monopole Resonance * Introduction * The Compressibility of nuclear matter from the GMR energies * Discussion * The Isoscalar Giant Quadrupole Resonance * General Trends In Medium-Heavy and Heavy Nuclei * The GQR In Light Nuclei * The Isoscalar 3- Strength, LEOR and HEOR * Isoscalar 4+ Strength * Miscellaneous; Isoscalar 1- and L > 4-Strength * The Electric Isovector Giant Resonances * The Isovector Giant Dipole Resonance: GDR * The Isovector Giant Monopole Resonances: IVGMR * The Isovector Quadrupole Resonance: IVGQR * The Effect of Ground State Deformation on the Shape of Giant Resonance: Microscopic Picture * Giant Resonances Built on Excited States * Introduction * Capture Reactions on Light Nuclei * Statistical decay of GDR γ Emission in Heavy Compound Systems * Introduction * Theoretical Predictions * Some Experimental Results * Summary and Outlook * Acknowledgements * General References * References

  14. Fano resonance and the hidden order in URu2 Si 2 probed by quasiparticle scattering spectroscopy*

    NASA Astrophysics Data System (ADS)

    Park, W. K.; Greene, L. H.; Bauer, E. D.; Tobash, P. H.; Ronning, F.; Lu, X.; Sarrao, J. L.; Thompson, J. D.

    2011-03-01

    The nature of the hidden order transition occurring at 17.5 K in URu 2 Si 2 remains puzzling despite intensive investigations over the past two and half decades. Recent experimental and theoretical developments render it a timely subject to probe the hidden order state using quasiparticle tunneling and scattering techniques. We report on the Fano resonance in pure and Rh-doped URu 2 Si 2 single crystals using point-contact spectroscopy. The conductance spectra reproducibly reveal asymmetric double peak structures slightly off-centered around zero bias with the two peaks merging well above the hidden order transition temperature. An analysis using the Fano resonance model in a Kondo lattice [1] shows that the conductance peaks arise from the hybridization gap opening. Our estimated gap size agrees well with those reported from other measurements. We will present experimental results over a wide parameter space including temperature and doping dependences and discuss their underlying physics. M. Maltseva, M. Dzero, and P. Coleman, Phys. Rev. Lett. 103, 206402 (2009). * The work at UIUC is supported by the U.S. DOE under Award Nos. DE-FG02-07ER46453 and DE-AC02-98CH10886, and the work at LANL is carried out under the auspices of the U.S. DOE, Office of Science.

  15. Vibrational resonance in Duffing systems with fractional-order damping.

    PubMed

    Yang, J H; Zhu, H

    2012-03-01

    The phenomenon of vibrational resonance (VR) is investigated in over- and under-damped Duffing systems with fractional-order damping. It is found that the factional-order damping can induce change in the number of the steady stable states and then lead to single- or double-resonance behavior. Compared with vibrational resonance in the ordinary systems, the following new results are found in the fractional-order systems. (1) In the overdamped system with double-well potential and ordinary damping, there is only one kind of single-resonance, whereas there are double-resonance and two kinds of single-resonance for the case of fractional-order damping. The necessary condition for these new resonance behaviors is the value of the fractional-order satisfies α > 1. (2) In the overdamped system with single-well potential and ordinary damping, there is no resonance, whereas there is a single-resonance for the case of fractional-order damping. The necessary condition for the new result is α > 1. (3) In the underdamped system with double-well potential and ordinary damping, there are double-resonance and one kind of single-resonance, whereas there are double-resonance and two kinds of single-resonance for the case of fractional-order damping. The necessary condition for the new single-resonance is α < 1. (4) In the underdamped system with single-well potential, there is at most a single-resonance existing for both the cases of ordinary and fractional-order damping. In the underdamped systems, varying the value of the fractional-order is equivalent to change the damping parameter for some cases.

  16. Doping effects on the hybridization gap and antiferromagnetic order in the Kondo semiconductor CeO s2A l10 studied by break-junction experiments

    NASA Astrophysics Data System (ADS)

    Kawabata, J.; Ekino, T.; Yamada, Y.; Okada, Y.; Sugimoto, A.; Muro, Y.; Takabatake, T.

    2017-01-01

    The Kondo semiconductors Ce T2A l10 (T =Ru and Os) exhibit antiferromagnetic (AFM) orders at unexpectedly high temperatures TN=27.0 and 28.5 K, respectively, whose mechanism remains in debate. We report the break-junction experiments on 4 f /5 d -hole and 5 d -electron doped CeO s2A l10 as well as nondoped CeR u2A l10 . The differential conductance spectra d I /d V for T =Os and Ru show three gap structures; two hybridization gaps V1, V2 and an AFM gap VAF, whose magnitudes for T =Os are 15 -50 % larger than for T =Ru . Doping of 4 f /5 d holes and 5 d electrons in CeO s2A l10 changes the d I /d V spectrum in very different ways. Nevertheless, in all cases, the suppression of V1 is well correlated with those of VAF and TN. Furthermore, the zero-bias conductance decreases on cooling below T* (>TN ) only in the doping region where V1 and VAF coexist. This fact indicates that the unusual AFM order is preceded by the decrease in the density of states in the presence of V1.

  17. Multi-orbital non-crossing approximation from maximally localized Wannier functions: the Kondo signature of copper phthalocyanine on Ag(100).

    PubMed

    Korytár, Richard; Lorente, Nicolás

    2011-09-07

    We have developed a multi-orbital approach to compute the electronic structure of a quantum impurity using the non-crossing approximation. The calculation starts with a mean-field evaluation of the system's electronic structure using a standard quantum chemistry code; here we use density functional theory (DFT). We transformed the one-electron structure into an impurity Hamiltonian by using maximally localized Wannier functions. Hence, we have developed a method to study the Kondo effect in systems based on an initial one-electron calculation. We have applied our methodology to a copper phthalocyanine molecule chemisorbed on Ag(100), and we have described its spectral function for three different cases where the molecule presents a single spin or two spins with ferro- and anti-ferromagnetic exchange couplings. We find that the use of broken-symmetry mean-field theories such as Kohn-Sham DFT cannot deal with the complexity of the spin of open-shell molecules on metal surfaces and extra modeling is needed.

  18. The spherical birdcage resonator

    NASA Astrophysics Data System (ADS)

    Harpen, Michael D.

    A description of the operation of a spherical resonator capable of producing a uniform magnetic induction throughout a spherical volume is presented. Simple closed-form expressions for the spectrum of resonant frequencies are derived for both the low-pass and the high-pass configuration of the resonator and are shown to compare favorably with observation in an experimental coil system. It is shown that the spherical resonator produces a uniform spherical field of view when used as a magnetic resonance imaging radiofrequency coil.

  19. Quantum critical behavior in an antiferromagnetic heavy-fermion Kondo lattice system (Ce{}_{1-x}La x )2Ir3Ge5

    NASA Astrophysics Data System (ADS)

    Khan, Rajwali; Mao, Qianhui; Wang, Hangdong; Yang, Jinhu; Du, Jianhua; Xu, Binjie; Zhou, Yuxing; Zhang, Yannan; Chen, Bing; Fang, Minghu

    2017-01-01

    Not Available Project supported by the National Basic Research Program of China (Grant Nos. 2016FYA0300402, 2015CB921004, and 2012CB821404) and the National Natural Science Foundation of China (Grant Nos. 11374261 and 11204059).

  20. Ovenized microelectromechanical system (MEMS) resonator

    SciTech Connect

    Olsson, Roy H; Wojciechowski, Kenneth; Kim, Bongsang

    2014-03-11

    An ovenized micro-electro-mechanical system (MEMS) resonator including: a substantially thermally isolated mechanical resonator cavity; a mechanical oscillator coupled to the mechanical resonator cavity; and a heating element formed on the mechanical resonator cavity.

  1. Optical Helmholtz resonators

    NASA Astrophysics Data System (ADS)

    Chevalier, Paul; Bouchon, Patrick; Haïdar, Riad; Pardo, Fabrice

    2014-08-01

    Helmholtz resonators are widely used acoustic components able to select a single frequency. Here, based on an analogy between acoustics and electromagnetism wave equations, we present an electromagnetic 2D Helmholtz resonator made of a metallic slit-box structure. At the resonance, the light is funneled in the λ/800 apertures, and is subsequently absorbed in the cavity. As in acoustics, there is no higher order of resonance, which is an appealing feature for applications such as photodetection or thermal emission. Eventually, we demonstrate that the slit is of capacitive nature while the box behaves inductively. We derive an analytical formula for the resonance wavelength, which does not rely on wave propagation and therefore does not depend on the permittivity of the material filling the box. Besides, in contrast with half-wavelength resonators, the resonance wavelength can be engineered by both the slit aspect ratio and the box area.

  2. Ultrasonic resonator for manipulation of bacteria

    NASA Astrophysics Data System (ADS)

    Schwarz, T.; Dual, J.

    2012-05-01

    Ultrasonic manipulation is a contactless and gentle method to manipulate a large number of particles. The method presented here exploits the advantage to simultaneously move bacteria away from a surface by means of acoustic radiation forces. The device for the manipulation consists of five layers (transducer, epoxy adhesive layer, carrier, fluid, reflector), stacked like a conventional planar resonator. The resonator behavior was simulated using the transfer matrix method (TMM). Validation of the model was realized with admittance measurements performed over a wide frequency range (100 kHz - 16 MHz). The TMM-model was used to optimize frequency, layer thickness and material of the resonator in order to find a combination with a high force potential gradient pointing away from the reflector surface into the fluid. The resonator has been experimentally tested with polystyrene particles (1 μm in diameter) which revealed a good matching with the TMM-model. First preliminary tests with Salmonella Thyphimurium have been done.

  3. Resonance splitting in gyrotropic ring resonators.

    PubMed

    Jalas, Dirk; Petrov, Alexander; Krause, Michael; Hampe, Jan; Eich, Manfred

    2010-10-15

    We present the theoretical concept of an optical isolator based on resonance splitting in a silicon ring resonator covered with a magneto-optical polymer cladding. For this task, a perturbation method is derived for the modes in the cylindrical coordinate system. A polymer magneto-optical cladding causing a 0.01 amplitude of the off-diagonal element of the dielectric tensor is assumed. It is shown that the derived resonance splitting of the clockwise and counterclockwise modes increases for smaller ring radii. For the ring with a radius of approximately 1.5μm, a 29GHz splitting is demonstrated. An integrated optical isolator with a 10μm geometrical footprint is proposed based on a critically coupled ring resonator.

  4. Nucleon Resonance Physics

    NASA Astrophysics Data System (ADS)

    Burkert, Volker D.

    2016-10-01

    Recent results of meson photo-production at the existing electron machines with polarized real photon beams and the measurement of polarization observables of the final state baryons have provided high precision data that led to the discovery of new excited nucleon and Δ states using multi-channel partial wave analyses procedures. The internal structure of several prominent excited states has been revealed employing meson electroproduction processes. On the theoretical front, lattice QCD is now predicting the baryon spectrum with very similar characteristics as the constituent quark model, and continuum QCD, such as is represented in the Dyson-Schwinger equations approach and in light front relativistic quark models, describes the non-perturbative behavior of resonance excitations at photon virtuality of Q^2 > 1.5 GeV^2. In this talk I discuss the need to continue a vigorous program of nucleon spectroscopy and the study of the internal structure of excited states as a way to reveal the effective degrees of freedom underlying the excited states and their dependence on the distance scale probed.

  5. Nucleon Resonance Physics

    SciTech Connect

    Burkert, Volker D.

    2016-07-25

    Recent results of meson photo-production at the existing electron machines with polarized real photon beams and the measurement of polarization observables of the final state baryons have provided high precision data that led to the discovery of new excited nucleon and $\\Delta$ states using multi-channel partial wave analyses procedures. The internal structure of several prominent excited states has been revealed employing meson electroproduction processes. On the theoretical front, lattice QCD is now predicting the baryon spectrum with very similar characteristics as the constituent quark model, and continuum QCD, such as is represented in the Dyson-Schwinger Equations approach and in light front relativistic quark models, describes the non-perturbative behavior of resonance excitations at photon virtuality of $Q^2 > 1.5GeV^2$. In this talk I discuss the need to continue a vigorous program of nucleon spectroscopy and the study of the internal structure of excited states as a way to reveal the effective degrees of freedom underlying the excited states and their dependence on the distance scale probed.

  6. Subwavelength resonant nanostructured films for sensing

    SciTech Connect

    Alvine, Kyle J.; Bernacki, Bruce E.; Suter, Jonathan D.; Bennett, Wendy D.; Edwards, Daniel L.; Mendoza, Albert

    2013-05-29

    We present a novel subwavelength nanostructure architecture that may be utilized for optical standoff sensing applications. The subwavelength structures are fabricated via a combination of nanoimprint lithography and metal sputtering to create metallic nanostructured films encased within a transparent media. The structures are based on the open ring resonator (ORR) architecture and have their analog in resonant LC circuits, which display a resonance frequency that is inversely proportional to the square root of the product of the inductance and capacitance. Therefore, any perturbation of the nanostructured films due to chemical or environmental effects can alter the inductive or capacitive behavior of the subwavelength features, which can shift the resonant frequency and provide an indication of the external stimulus. This shift in resonance can be interrogated remotely either actively using either laser illumination or passively using hyperspectral or multispectral sensing. These structures may be designed to be either anisotropic or isotropic, which can also provide polarization-sensitive interrogation. Due to the nanometer-scale of the structures, they can be tailored to be optically responsive in the visible or near infrared spectrum with a highly reflective resonant peak that is dependent solely on structural dimensions and material characteristics. We present experimental measurements of the optical response of these structures as a function of wavelength, polarization, and incident angle demonstrating the resonant effect in the near infrared region. Numerical modeling data showing the effect of different fabrication parameters such as structure parameters are also discussed.

  7. Spectroscopic studies of individual plasmon resonant nanoparticles

    NASA Astrophysics Data System (ADS)

    Mock, Jack J.; Smith, David R.; Barbic, Mladen; Oldenburg, Steven J.; Schultz, David A.; Schultz, Sheldon

    2003-11-01

    We present a detailed description of the apparatus and techniques that we have utilized in our experimental study of individual plas on resonant nanoparticles,along with a brief description of some major results. The apparatus consists of a spectroscopic system combined with a modified darkfield microscope, which enables the user to sequentially select individual resonant nanostructures in the microscopic field of view for spectroscopic study. Plasmon resonant nanostructures scatter light elastically,and typically have very large scattering cross-sections at their resonant optical wavelengths. In general, spectra can be obtained with acquisition times between .1 to 30 seconds,and color images can be captured using consumer digital color cameras. Spheres,tetrahedrons,and pentagonal platelets were fabricated using colloidal chemistry techniques. To produce highly anisotropic structures such as nanorods and "barbells", templates were used. Many of these nanostructures have been individually spectroscopically characterized,and their spectra correlated with their shape and size as determined by transmission electron icroscope (TEM). The unique shape,size, composition,and dielectric surroundings of the individual plasmon resonant nanostructures determine their plasmon resonant behavior. We will show how the composition of the substrate on which the particles are immobilized and the dielectric of the surrounding medium have a significant effect on the plasmon resonance of the individual particles.

  8. Designing Multipolar Resonances in Dielectric Metamaterials

    PubMed Central

    Butakov, Nikita A.; Schuller, Jon A.

    2016-01-01

    Dielectric resonators form the building blocks of nano-scale optical antennas and metamaterials. Due to their multipolar resonant response and low intrinsic losses they offer design flexibility and high-efficiency performance. These resonators are typically described in terms of a spherical harmonic decomposition with Mie theory. In experimental realizations however, a departure from spherical symmetry and the use of high-index substrates leads to new features appearing in the multipolar response. To clarify this behavior, we present a systematic experimental and numerical characterization of Silicon disk resonators. We demonstrate that for disk resonators on low-index quartz substrates, the electric and magnetic dipole modes are easily identifiable across a wide range of aspect-ratios, but that higher order peaks cannot be unambiguously associated with any specific multipolar mode. On high-index Silicon substrates, even the fundamental dipole modes do not have a clear association. When arranged into arrays, resonances are shifted and pronounced preferential forward and backward scattering conditions appear, which are not as apparent in individual resonators and may be associated with interference between multipolar modes. These findings present new opportunities for engineering the multipolar scattering response of dielectric optical antennas and metamaterials, and provide a strategy for designing nano-optical components with unique functionalities. PMID:27929038

  9. Designing Multipolar Resonances in Dielectric Metamaterials

    NASA Astrophysics Data System (ADS)

    Butakov, Nikita A.; Schuller, Jon A.

    2016-12-01

    Dielectric resonators form the building blocks of nano-scale optical antennas and metamaterials. Due to their multipolar resonant response and low intrinsic losses they offer design flexibility and high-efficiency performance. These resonators are typically described in terms of a spherical harmonic decomposition with Mie theory. In experimental realizations however, a departure from spherical symmetry and the use of high-index substrates leads to new features appearing in the multipolar response. To clarify this behavior, we present a systematic experimental and numerical characterization of Silicon disk resonators. We demonstrate that for disk resonators on low-index quartz substrates, the electric and magnetic dipole modes are easily identifiable across a wide range of aspect-ratios, but that higher order peaks cannot be unambiguously associated with any specific multipolar mode. On high-index Silicon substrates, even the fundamental dipole modes do not have a clear association. When arranged into arrays, resonances are shifted and pronounced preferential forward and backward scattering conditions appear, which are not as apparent in individual resonators and may be associated with interference between multipolar modes. These findings present new opportunities for engineering the multipolar scattering response of dielectric optical antennas and metamaterials, and provide a strategy for designing nano-optical components with unique functionalities.

  10. Quantum processes in resonators with moving walls

    NASA Technical Reports Server (NTRS)

    Klimov, A. B.; Dodonov, V. V.

    1993-01-01

    The behavior of an electromagnetic field in an ideal cavity with an oscillating boundary is considered in the resonance long-time limit. The rates of photon creation from the vacuum and thermal states are evaluated. The squeezing coefficients for the field modes are found, as well as the backward reaction of the field on the vibrating wall.

  11. CBERS Satellites: Resonant Orbital Motions in LEO Region

    NASA Astrophysics Data System (ADS)

    Vilhena de Moraes, Rodolpho; Sampaio, J. C.; da Silva Fernandes, S.; Wnuk, E.

    2013-05-01

    Abstract (2,250 Maximum Characters): The space between the Earth and the Moon has several artificial satellites and space debris in some resonance. Synchronous satellites in circular or elliptical orbits have been studied in literature, including the analysis of resonant orbits characterizing the dynamics of these satellites. In general, some resonant angles associated to the exact resonance are considered in the numerical integration, with the purpose to describe the resonance defined by the commensurability between the mean motion of the object and the Earth’s rotation angular velocity. However, the tesseral harmonics Jlm produce multiple resonances in the exact resonance and in the neighborhood of the exact resonance, and, some disturbances in the orbital motions of objects are not described. In this work, the TLE (Two-Line Elements) of the NORAD (North American Defense) are studied observing the resonant objects orbiting the Earth in LEO (Low Earth Orbit) region. Analyzing the cataloged objects, the CBERS satellites are studied observing resonance effects which compose your orbits. The time behavior of the orbital elements, resonant period and resonant angles are considered and possible regular and irregular motions are analyzed. About 60 space debris produced by the CBERS-1 satellite mission are studied analyzing the reentry of these objects in the Planet.

  12. Influence of the electron spin resonance saturation on the power sensitivity of cryogenic sapphire resonators

    SciTech Connect

    Giordano, Vincent Grop, Serge; Bourgeois, Pierre-Yves; Kersalé, Yann; Rubiola, Enrico

    2014-08-07

    Here, we study the paramagnetic ions behavior in presence of a strong microwave electromagnetic field sustained inside a cryogenic sapphire whispering gallery mode resonator. The high frequency measurement resolution that can be now achieved by comparing two Cryogenic Sapphire Oscillators (CSOs) permit to observe clearly the non-linearity of the resonator power sensitivity. These observations that, in turn, allow us to optimize the CSO operation are well explained by the electron spin resonance saturation of the paramagnetic impurities contained in the sapphire crystal.

  13. Exploring the Outer Neptune Resonances: Constraints on Solar System Evolution

    NASA Astrophysics Data System (ADS)

    Pike, Rosemary E.; Kavelaars, JJ; Shankman, Cory J.; Petit, Jean-Marc; Brett, Gladman; Volk, Kat; Alexandersen, Mike

    2015-11-01

    The long-term evolution of objects in the outer n:1 resonances with Neptune provide clues to the evolutionary history of the Solar System. Based on 4 objects with semi-major axes near the 5:1 resonance, we estimate a substantial and previously unrecognized population of objects, perhaps more significant than the population in the 3:2 (Plutino) resonance. These external resonances are largely unexplored in both observations and dynamical simulations. However, understanding the characteristics and trapping history for objects in these populations is critical for constraining the dynamical history of the solar system. The 4 objects detected in the Canada-France Ecliptic Plane Survey (CFEPS) were classified using dynamical integrations. Three are resonant, and the fourth appears to be a resonance diffusion object, part of a population which exited the resonance through chaotic diffusion. The 3 resonant objects are taken to be representative of the resonant population, so by using these detections and the CFEPS characterization (pointings and detection limits) we calculate a population estimate for this resonance at ~1900(+3300 -1400) objects with Hg<8 [Pike et al. 2015]. This is at least as large as the Plutinos (3:2 resonance) at 90% confidence. The small number of detected objects results in such a large population estimate due to the numerous biases against detecting objects with semimajor axes at ~88AU. The dynamical behavior of the known objects, suggests that the trapping mechanism for the 5:1 resonance is resonance sticking from the scattering objects. Based on our results from the 5:1 resonance, we have begun a project to examine the long term evolution of the other n:1 resonances to determine the importance of resonance diffusion and transfer between libration islands among the scattering-captured members of those populations.

  14. Casimir effect on graphene resonator

    NASA Astrophysics Data System (ADS)

    Inui, Norio

    2016-03-01

    We theoretically investigated the influence of the Casimir effect on mechanical properties of a graphene resonator, where a graphene sheet is located in parallel with a perfectly conducting plate. The Casimir force arising from this effect strongly attracts a graphene sheet to a perfectly conducting plate and increases the tension of a graphene sheet as the separation distance between them decreases. The maximum vertical displacement of a graphene sheet to the substrate increases obeying a power law of a separation distance with an exponent of 4/3 as the separation distance decreases. For small separation distances, the Casimir force is excessively strong for the graphene sheet to maintain a free-standing shape, consequently resulting in the adhesion of the sheet to the substrate below a critical separation distance. The resonant frequency increases over a wide range as the separation distance decreases for large separation distances. However, it then rapidly decreases for small separations and converges to zero at a critical separation. These various behaviors enable the control of a graphene resonator.

  15. Resonant Versus Anti-Resonant Tunneling at Carbon Nanotube A-B-A Heterostructures

    NASA Technical Reports Server (NTRS)

    Mingo, N.; Yang, Liu; Han, Jie; Anantram, M. P.

    2001-01-01

    Narrow antiresonances going to zero transmission are found to occur for general (2n,0)(n,n)(2n,0) carbon nanotube heterostructures, whereas the complementary configuration, (n,n)(2n,0)(n,n), displays simple resonant tunneling behaviour. We compute examples for different cases, and give a simple explanation for the appearance of antiresonances in one case but not in the other. Conditions and ranges for the occurrence of these different behaviors are stated. The phenomenon of anti-resonant tunneling, which has passed unnoticed in previous studies of nanotube heterostructures, adds up to the rich set of behaviors available to nanotube based quantum effect devices.

  16. Large mode radius resonators

    NASA Technical Reports Server (NTRS)

    Harris, Michael R.

    1987-01-01

    Resonator configurations permitting operation with large mode radius while maintaining good transverse mode discrimination are considered. Stable resonators incorporating an intracavity telescope and unstable resonator geometries utilizing an output coupler with a Gaussian reflectivity profile are shown to enable large radius single mode laser operation. Results of heterodyne studies of pulsed CO2 lasers with large (11mm e sup-2 radius) fundamental mode sizes are presented demonstrating minimal frequency sweeping in accordance with the theory of laser-induced medium perturbations.

  17. The Use and Evaluation of Scaffolding, Student Centered-Learning, Behaviorism, and Constructivism to Teach Nuclear Magnetic Resonance and IR Spectroscopy in a Two-Semester Organic Chemistry Course

    ERIC Educational Resources Information Center

    Livengood, Kimberly; Lewallen, Denver W.; Leatherman, Jennifer; Maxwell, Janet L.

    2012-01-01

    Since 2002, infrared spectroscopy (IR) and nuclear magnetic resonance (NMR) spectrometry have been introduced at the beginning of the first-semester organic chemistry lab course at this university. Starting in 2008, each individual student was given 20 unique homework problems that consisted of multiple-choice [superscript 1]H NMR and IR problems…

  18. Emergent behavior in strongly correlated electron systems

    NASA Astrophysics Data System (ADS)

    Pines, David

    2016-09-01

    I describe early work on strongly correlated electron systems (SCES) from the perspective of a theoretical physicist who, while a participant in their reductionist top-down beginnings, is now part of the paradigm change to a bottom-up ‘emergent’ approach with its focus on using phenomenology to find the organizing principles responsible for their emergent behavior disclosed by experiment—and only then constructing microscopic models that incorporate these. After considering the organizing principles responsible for the emergence of plasmons, quasiparticles, and conventional superconductivity in SCES, I consider their application to three of SCES’s sister systems, the helium liquids, nuclei, and the nuclear matter found in neutron stars. I note some recent applications of the random phase approximation and examine briefly the role that paradigm change is playing in two central problems in our field: understanding the emergence and subsequent behavior of heavy electrons in Kondo lattice materials; and finding the mechanism for the unconventional superconductivity found in heavy electron, organic, cuprate, and iron-based materials.

  19. Emergent behavior in strongly correlated electron systems.

    PubMed

    Pines, David

    2016-09-01

    I describe early work on strongly correlated electron systems (SCES) from the perspective of a theoretical physicist who, while a participant in their reductionist top-down beginnings, is now part of the paradigm change to a bottom-up 'emergent' approach with its focus on using phenomenology to find the organizing principles responsible for their emergent behavior disclosed by experiment-and only then constructing microscopic models that incorporate these. After considering the organizing principles responsible for the emergence of plasmons, quasiparticles, and conventional superconductivity in SCES, I consider their application to three of SCES's sister systems, the helium liquids, nuclei, and the nuclear matter found in neutron stars. I note some recent applications of the random phase approximation and examine briefly the role that paradigm change is playing in two central problems in our field: understanding the emergence and subsequent behavior of heavy electrons in Kondo lattice materials; and finding the mechanism for the unconventional superconductivity found in heavy electron, organic, cuprate, and iron-based materials.

  20. Mechanical Resonances of Helically Coiled Carbon Nanowires

    PubMed Central

    Saini, D.; Behlow, H.; Podila, R.; Dickel, D.; Pillai, B.; Skove, M. J.; Serkiz, S. M.; Rao, A. M.

    2014-01-01

    Despite their wide spread applications, the mechanical behavior of helically coiled structures has evaded an accurate understanding at any length scale (nano to macro) mainly due to their geometrical complexity. The advent of helically coiled micro/nanoscale structures in nano-robotics, nano-inductors, and impact protection coatings has necessitated the development of new methodologies for determining their shear and tensile properties. Accordingly, we developed a synergistic protocol which (i) integrates analytical, numerical (i.e., finite element using COMSOL®) and experimental (harmonic detection of resonance; HDR) methods to obtain an empirically validated closed form expression for the shear modulus and resonance frequency of a singly clamped helically coiled carbon nanowire (HCNW), and (ii) circumvents the need for solving 12th order differential equations. From the experimental standpoint, a visual detection of resonances (using in situ scanning electron microscopy) combined with HDR revealed intriguing non-planar resonance modes at much lower driving forces relative to those needed for linear carbon nanotube cantilevers. Interestingly, despite the presence of mechanical and geometrical nonlinearities in the HCNW resonance behavior the ratio of the first two transverse modes f2/f1 was found to be similar to the ratio predicted by the Euler-Bernoulli theorem for linear cantilevers. PMID:24986377