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Sample records for kondo resonance behaviors

  1. Lateral manipulation and interplay of local Kondo resonances in a two-impurity Kondo system

    NASA Astrophysics Data System (ADS)

    Ren, Jindong; Wu, Xu; Guo, Haiming; Pan, Jinbo; Du, Shixuan; Luo, Hong-Gang; Gao, Hong-Jun

    2015-08-01

    The atomic-scale spatial relationship of a two-impurity Kondo system has been determined at varying lateral distance by scanning tunneling microscopy (STM) and spectroscopy. The localized spins of two cobalt magnetic adatoms that are placed on different electrodes of an STM form two individual Kondo singlet states, each showing quite different Kondo coupling, i.e., the tip-Kondo with low Kondo temperature and the sample-Kondo with high Kondo temperature. The differential conductance dI/dV spectra show the continuous changes of the resonance peak feature when approaching the Kondo tip laterally to the local sample-Kondo impurity on the surface. The result indicates a notable interplay between these two Kondo systems. We propose a convolution model based on the q factor of the sample-Kondo (qs) and tip-Kondo (qt) to interpret the change of various tunneling channels and the evolution of the experimental spectra.

  2. Lateral manipulation and interplay of local Kondo resonances in a two-impurity Kondo system

    SciTech Connect

    Ren, Jindong; Wu, Xu; Guo, Haiming Pan, Jinbo; Du, Shixuan; Gao, Hong-Jun; Luo, Hong-Gang

    2015-08-17

    The atomic-scale spatial relationship of a two-impurity Kondo system has been determined at varying lateral distance by scanning tunneling microscopy (STM) and spectroscopy. The localized spins of two cobalt magnetic adatoms that are placed on different electrodes of an STM form two individual Kondo singlet states, each showing quite different Kondo coupling, i.e., the tip-Kondo with low Kondo temperature and the sample-Kondo with high Kondo temperature. The differential conductance dI/dV spectra show the continuous changes of the resonance peak feature when approaching the Kondo tip laterally to the local sample-Kondo impurity on the surface. The result indicates a notable interplay between these two Kondo systems. We propose a convolution model based on the q factor of the sample-Kondo (q{sub s}) and tip-Kondo (q{sub t}) to interpret the change of various tunneling channels and the evolution of the experimental spectra.

  3. Nuclear magnetic resonance in Kondo lattice systems.

    PubMed

    Curro, Nicholas J

    2016-06-01

    Nuclear magnetic resonance has emerged as a vital tool to explore the fundamental physics of Kondo lattice systems. Because nuclear spins experience two different hyperfine couplings to the itinerant conduction electrons and to the local f moments, the Knight shift can probe multiple types of spin correlations that are not accessible via other techniques. The Knight shift provides direct information about the onset of heavy electron coherence and the emergence of the heavy electron fluid.

  4. Kondo effect and non-Fermi-liquid behavior in Dirac and Weyl semimetals

    NASA Astrophysics Data System (ADS)

    Principi, Alessandro; Vignale, Giovanni; Rossi, E.

    2015-07-01

    We study the Kondo effect in three-dimensional (3D) Dirac materials and Weyl semimetals. We find the scaling of the Kondo temperature with respect to the doping n and the coupling J between the moment of the magnetic impurity and the carriers of the semimetal. We consider the interplay of long-range scalar disorder and Kondo screening and find that it causes the Kondo effect to be characterized not by a Kondo temperature, but by a distribution of Kondo temperatures with features that cause the appearance of strong non-Fermi-liquid behavior. We then consider the effect of Kondo screening, and of the interplay of Kondo screening and long-range scalar disorder, on the transport properties of Weyl semimetals. Finally, we compare the properties of the Kondo effect in 3D and 2D Dirac materials such as graphene and topological insulators.

  5. Kondo Resonance of a Co Atom Exchange Coupled to a Ferromagnetic Tip

    NASA Astrophysics Data System (ADS)

    Choi, D.-J.; Guissart, S.; Ormaza, M.; Bachellier, N.; Bengone, O.; Simon, P.; Limot, L.

    2016-10-01

    The Kondo effect of a Co atom on Cu(100) was investigated with a low-temperature scanning tunneling microscope using a monoatomically sharp nickel tip. Upon a tip-Co contact, the differential conductance spectra exhibit a spin-split asymmetric Kondo resonance. The computed ab initio value of the exchange coupling is too small to suppress the Kondo effect, but sufficiently large to produce the splitting observed. A quantitative analysis of the line shape using the numerical renormalization group technique indicates that the junction spin polarization is weak.

  6. Blocking transport resonances via Kondo many-body entanglement in quantum dots

    NASA Astrophysics Data System (ADS)

    Niklas, Michael; Smirnov, Sergey; Mantelli, Davide; Margańska, Magdalena; Nguyen, Ngoc-Viet; Wernsdorfer, Wolfgang; Cleuziou, Jean-Pierre; Grifoni, Milena

    2016-08-01

    Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we show another side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic co-tunnelling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global SU(2) \\xotime SU(2) symmetry of a nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin.

  7. Blocking transport resonances via Kondo many-body entanglement in quantum dots

    NASA Astrophysics Data System (ADS)

    Niklas, Michael; Smirnov, Sergey; Mantelli, Davide; Margańska, Magdalena; Nguyen, Ngoc-Viet; Wernsdorfer, Wolfgang; Cleuziou, Jean-Pierre; Grifoni, Milena

    2016-08-01

    Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we show another side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic co-tunnelling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global SU(2) ⨂ SU(2) symmetry of a nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin.

  8. Self-sustained oscillations in nanoelectromechanical systems induced by Kondo resonance

    NASA Astrophysics Data System (ADS)

    Song, Taegeun; Kiselev, Mikhail N.; Kikoin, Konstantin; Shekhter, Robert I.; Gorelik, Leonid Y.

    2014-03-01

    We investigate the instability and dynamical properties of nanoelectromechanical systems represented by a single-electron device containing movable quantum dots attached to a vibrating cantilever via asymmetric tunnel contacts. The Kondo resonance in electron tunneling between the source and shuttle facilitates self-sustained oscillations originating from the strong coupling of mechanical and electronic/spin degrees of freedom. We analyze a stability diagram for the two-channel Kondo shuttling regime due to limitations given by the electromotive force acting on a moving shuttle, and find that the saturation oscillation amplitude is associated with the retardation effect of the Kondo cloud. The results shed light on possible ways to experimentally realize the Kondo-cloud dynamical probe by using high mechanical dissipation tunability as well as supersensitive detection of mechanical displacement.

  9. Sub-molecular modulation of a 4f driven Kondo resonance by surface-induced asymmetry

    PubMed Central

    Warner, Ben; El Hallak, Fadi; Atodiresei, Nicolae; Seibt, Philipp; Prüser, Henning; Caciuc, Vasile; Waters, Michael; Fisher, Andrew J.; Blügel, Stefan; van Slageren, Joris; Hirjibehedin, Cyrus F.

    2016-01-01

    Coupling between a magnetic impurity and an external bath can give rise to many-body quantum phenomena, including Kondo and Hund's impurity states in metals, and Yu-Shiba-Rusinov states in superconductors. While advances have been made in probing the magnetic properties of d-shell impurities on surfaces, the confinement of f orbitals makes them difficult to access directly. Here we show that a 4f driven Kondo resonance can be modulated spatially by asymmetric coupling between a metallic surface and a molecule containing a 4f-like moment. Strong hybridization of dysprosium double-decker phthalocyanine with Cu(001) induces Kondo screening of the central magnetic moment. Misalignment between the symmetry axes of the molecule and the surface induces asymmetry in the molecule's electronic structure, spatially mediating electronic access to the magnetic moment through the Kondo resonance. This work demonstrates the important role that molecular ligands have in mediating electronic and magnetic coupling and in accessing many-body quantum states. PMID:27666413

  10. Sub-molecular modulation of a 4f driven Kondo resonance by surface-induced asymmetry

    NASA Astrophysics Data System (ADS)

    Warner, Ben; El Hallak, Fadi; Atodiresei, Nicolae; Seibt, Philipp; Pruser, Henning; Caciuc, Vasile; Waters, Michael; Fisher, Andrew J.; Blugel, Stefan; van Slageren, Joris; Hirjibehedin, Cyrus F.

    Coupling between a magnetic impurity and an external bath can give rise to many-body quantum phenomena, including Kondo and Hund's Impurity states in metals, and Yu-Shiba-Rusinov states in superconductors. While advances have been made in probing the magnetic properties of d-shell impurities on surfaces, the confinement of f orbitals makes them much more difficult to access directly. Here we show that a 4f driven Kondo resonance can be modulated spatially by asymmetric coupling between a metallic surface and a molecule containing a 4f-like moment. Strong hybridisation of dysprosium double-decker phthalocyanine (DyPc2) with Cu(001) induces Kondo screening of the central magnetic moment. Misalignment between the symmetry axes of the molecule and the surface induces asymmetry in the molecule's electronic structure, spatially mediating electronic access to the magnetic moment through the Kondo resonance. This work demonstrates the important role that molecular ligands play in mediating electronic and magnetic coupling and in accessing many-body quantum states.

  11. Blocking transport resonances via Kondo many-body entanglement in quantum dots.

    PubMed

    Niklas, Michael; Smirnov, Sergey; Mantelli, Davide; Margańska, Magdalena; Nguyen, Ngoc-Viet; Wernsdorfer, Wolfgang; Cleuziou, Jean-Pierre; Grifoni, Milena

    2016-01-01

    Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we show another side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic co-tunnelling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global SU(2) ⊗ SU(2) symmetry of a nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin. PMID:27526870

  12. Blocking transport resonances via Kondo many-body entanglement in quantum dots

    PubMed Central

    Niklas, Michael; Smirnov, Sergey; Mantelli, Davide; Margańska, Magdalena; Nguyen, Ngoc-Viet; Wernsdorfer, Wolfgang; Cleuziou, Jean-Pierre; Grifoni, Milena

    2016-01-01

    Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we show another side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic co-tunnelling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global SU(2) ⊗ SU(2) symmetry of a nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin. PMID:27526870

  13. Intramolecularly resolved Kondo resonance of high-spin Fe (II ) -porphyrin adsorbed on Au ( 111 )

    NASA Astrophysics Data System (ADS)

    Wang, Weihua; Pang, Rui; Kuang, Guowen; Shi, Xingqiang; Shang, Xuesong; Liu, Pei Nian; Lin, Nian

    2015-01-01

    Using cryogenic scanning tunneling microscopy, we measured the electronic states and Kondo resonance of single Fe (II ) -porphyrin molecules adsorbed on a Au ( 111 ) surface with intramolecular resolution. We found that the Fe (II ) ion introduces a spin-polarized molecular state near the Fermi level. Tunneling spectroscopy revealed that this state gives rise to Kondo resonance exhibiting characteristics different from those of the Fe (II ) spin state. Spin-polarized density functional theory calculations revealed that the molecule was weakly adsorbed on the surface, yet still switches its spin configuration from S =1 to2 . The spin switching was found to be driven by three effects: a structural distortion of the macrocyclic ring from planar to saddle shaped, a weak chemical bonding between the Fe and the Au surface atom underneath, and weakened Fe-N bonds due to Au ( 111 ) -molecule charge transfer.

  14. Electron-vibration interaction in the presence of a switchable Kondo resonance realized in a molecular junction.

    PubMed

    Rakhmilevitch, D; Korytár, R; Bagrets, A; Evers, F; Tal, O

    2014-12-01

    The interaction of individual electrons with vibrations has been extensively studied. However, the nature of electron-vibration interaction in the presence of many-body electron correlations such as a Kondo state has not been fully investigated. Here, we present transport measurements on a Copper-phthalocyanine molecule, suspended between two silver electrodes in a break-junction setup. Our measurements reveal both zero bias and satellite conductance peaks, which are identified as Kondo resonances with a similar Kondo temperature. The relation of the satellite peaks to electron-vibration interaction is corroborated using several independent spectroscopic indications, as well as ab initio calculations. Further analysis reveals that the contribution of vibration-induced inelastic current is significant in the presence of a Kondo resonance. PMID:25526145

  15. Fano Antiresonance and Kondo Resonance for Electronic Transport Through a Laterally Coupled Carbon-Nanotube Quantum-Dot System

    NASA Astrophysics Data System (ADS)

    Huo, Dong-Ming

    2015-10-01

    We present nonequilibrium Green function calculations for electronic transport through a laterally coupled carbon-nanotube quantum-dot system. In this system, a one-dimensional double carbon nanotube quantum dot attached to polarised electrodes forms a main channel for electronic tunnelling. Each carbon nanotube quantum dot in the main channel couples to a dangling carbon nanotube quantum dot. Then, the conductance spectrum is calculated. The insulating band and resonance peak in this spectrum, due to Fano antiresonance and Kondo resonance, are discussed. The intradot electron's Coulomb interaction effect on the insulating band is also investigated. By controlling the coupling coefficient between the quantum dots, we can realise mutual transformation between Kondo resonance and Fano antiresonance at the Fermi level. The spin-orbit coupling and magnetic field's influence on the Kondo resonance peak are discussed in detail. Finally, spin magnetic moment and orbital magnetic moment of electrons in the quantum dot by applying parallel magnetic field are also predicted.

  16. Low-temperature behavior of transmission phase shift across a Kondo correlated quantum dot

    NASA Astrophysics Data System (ADS)

    Takada, S.; Yamamoto, M.; Bäuerle, C.; Alex, A.; von Delft, J.; Ludwig, A.; Wieck, A. D.; Tarucha, S.

    2016-08-01

    We study the transmission phase shift across a Kondo correlated quantum dot in a GaAs heterostructure at temperatures below the Kondo temperature (T Kondo singlet ground state. Our device is tuned such that the ratio Γ /U of level width Γ to charging energy U is quite large (≲0.5 rather than ≪1 ). This situation is commonly used in GaAs quantum dots to ensure Kondo temperatures large enough (≃ 100 mK here) to be experimentally accessible; however, it also implies that charge fluctuations are more pronounced than typically assumed in theoretical studies focusing on the regime Γ /U ≪1 needed to ensure a well-defined local moment. Our measured phase evolves monotonically by π across the two Coulomb peaks, but without being locked at π /2 in the Kondo valley for T ≪TK , due to a significant influence of large Γ /U . Only when Γ /U is reduced sufficiently does the phase start to be locked around π /2 and develops into a plateau at π /2 . Our observations are consistent with numerical renormalization group calculations, and can be understood as a direct consequence of the Friedel sum rule that relates the transmission phase shift to the local occupancy of the dot, and thermal average of a transmission coefficient through a resonance level near the Fermi energy.

  17. Mapping itinerant electrons around Kondo impurities.

    PubMed

    Prüser, H; Wenderoth, M; Weismann, A; Ulbrich, R G

    2012-04-20

    We investigate single Fe and Co atoms buried below a Cu(100) surface using low temperature scanning tunneling spectroscopy. By mapping the local density of states of the itinerant electrons at the surface, the Kondo resonance near the Fermi energy is analyzed. Probing bulk impurities in this well-defined scattering geometry allows separating the physics of the Kondo system and the measuring process. The line shape of the Kondo signature shows an oscillatory behavior as a function of depth of the impurity as well as a function of lateral distance. The oscillation period along the different directions reveals that the spectral function of the itinerant electrons is anisotropic. PMID:22680744

  18. Interference effects and Fano resonance in transport across a two dot system in the Kondo regime

    NASA Astrophysics Data System (ADS)

    Sztenkiel, D.; Swirkowicz, R.

    2007-09-01

    Transport across a double dot system of a special geometry with two channels accessible for tunneling electrons is theoretically studied in a region of low temperatures corresponding to the Kondo regime, and interference effects are analyzed. The spectral function and the linear conductance are calculated using the Green function formalism based on the equation of motion method. It is shown that interference processes strongly influence the spectral function. Moreover, due to interference effects the conductance, which is close to zero in a low energy region, shows at higher gate voltages a well defined Fano resonance. A development of the Fano peak as the system undergoes a gradual transition from the serial configuration to the geometry with two dots partially connected to both electrodes is demonstrated. The position and intensity of the Fano resonance strongly depend on the inter-dot tunneling rate. The influence of temperature on the resonance is also discussed.

  19. Emergent Kondo Lattice Behavior in Iron-Based Superconductors A Fe2As2 (A =K , Rb, Cs)

    NASA Astrophysics Data System (ADS)

    Wu, Y. P.; Zhao, D.; Wang, A. F.; Wang, N. Z.; Xiang, Z. J.; Luo, X. G.; Wu, T.; Chen, X. H.

    2016-04-01

    Here, we experimentally study the origin of d -electron heavy fermion (HF) behavior in iron-based superconductors (FeSCs) A Fe2As2 (A =K , Rb, Cs). Nuclear magnetic resonance on 75As reveals a universal coherent-incoherent crossover with a characteristic temperature T*. Below T*, a so-called "Knight shift anomaly" is first observed in FeSCs, which exhibits a scaling behavior similar to f -electron HF materials. Furthermore, the scaling rule also regulates the manifestation of magnetic fluctuation. These results undoubtedly support an emergent Kondo lattice scenario for the d -electron HF behavior, which qualifies the A Fe2As2 (A =K , Rb, Cs) as d -electron HF superconductors.

  20. Emergent Kondo Lattice Behavior in Iron-Based Superconductors AFe_{2}As_{2} (A=K, Rb, Cs).

    PubMed

    Wu, Y P; Zhao, D; Wang, A F; Wang, N Z; Xiang, Z J; Luo, X G; Wu, T; Chen, X H

    2016-04-01

    Here, we experimentally study the origin of d-electron heavy fermion (HF) behavior in iron-based superconductors (FeSCs) AFe_{2}As_{2} (A=K, Rb, Cs). Nuclear magnetic resonance on ^{75}As reveals a universal coherent-incoherent crossover with a characteristic temperature T^{*}. Below T^{*}, a so-called "Knight shift anomaly" is first observed in FeSCs, which exhibits a scaling behavior similar to f-electron HF materials. Furthermore, the scaling rule also regulates the manifestation of magnetic fluctuation. These results undoubtedly support an emergent Kondo lattice scenario for the d-electron HF behavior, which qualifies the AFe_{2}As_{2} (A=K, Rb, Cs) as d-electron HF superconductors. PMID:27104721

  1. Strongly correlated plexcitonics: evolution of the Fano resonance in the presence of Kondo correlations.

    PubMed

    Goker, A

    2015-05-01

    We study the optical absorption of a system consisting of a diatomic molecule that exhibits strong electron correlations coupled to metal nanoparticles possessing plasmon resonances by invoking the time-dependent non-crossing approximation. We investigate the evolution of the Fano resonance arising from the plasmon-exciton coupling when both atoms are Coulomb blockaded. We found that the Fano resonance rapidly dwindles as the ambient temperature exceeds the Kondo temperature of the singly occupied discrete state with higher energy and vanishes entirely at elevated temperatures. Our results show that even boosting the plasmon-exciton coupling above this temperature scale fails to revive the Fano resonance. We propose a microscopic model that accounts for these results. We suggest that a possible remedy for observation of the Fano resonance at high ambient temperatures is to position the singly occupied discrete state with the higher energy as close as possible to the Fermi level of the contacts while keeping the emitter resonance constant to prevent the merger of the Fano and plasmon resonances. PMID:25858207

  2. Real-space imaging of Kondo screening in a two-dimensional O₂ lattice.

    PubMed

    Jiang, Ying; Zhang, Y N; Cao, J X; Wu, R Q; Ho, W

    2011-07-15

    Kondo lattice systems can exhibit unusual many-body behaviors that result from the interplay between onsite Kondo screening and intersite coupling. We used scanning tunneling microscopy to image the Kondo resonance in a nonconventional Kondo lattice formed by self-assembled oxygen (O(2)) molecules, which are paramagnetic, on the gold reconstructed surface [Au(110)-1×2]. The interplay between the intermolecular coupling for molecules adsorbed along chains and the onsite Kondo effect leads to the coexistence of both local and nonlocal Kondo screening at the atomic level. The latter provides evidence for collective deconfinement of magnetization induced in Au, whereas the former shows local "hybridization" between the Kondo clouds of nearest-neighbor O(2) molecules.

  3. Magnetic ordering and non-Fermi-liquid behavior in the multichannel Kondo-lattice model

    NASA Astrophysics Data System (ADS)

    Irkhin, Valentin Yu.

    2016-05-01

    Scaling equations for the Kondo lattice in the paramagnetic and magnetically ordered phases are derived to next-leading order with account of spin dynamics. The results are applied to describe various mechanisms of the non-Fermi-liquid (NFL) behavior in the multichannel Kondo-lattice model where a fixed point occurs in the weak-coupling region. The corresponding temperature dependences of electronic and magnetic properties are discussed. The model describes naturally formation of a magnetic state with soft boson mode and small moment value. An important role of Van Hove singularities in the magnon spectral function is demonstrated. The results are rather sensitive to the type of magnetic ordering and space dimensionality, the conditions for NFL behavior being more favorable in the antiferromagnetic and 2D cases.

  4. Kondo-type behavior of the Ru4 + lattice in LaCu3Ru4O12

    NASA Astrophysics Data System (ADS)

    Riegg, S.; Widmann, S.; Meir, B.; Sterz, S.; Günther, A.; Büttgen, N.; Ebbinghaus, S. G.; Reller, A.; von Nidda, H.-A. Krug; Loidl, A.

    2016-03-01

    Rare d -electron-derived heavy-fermion properties of the solid-solution series LaCu3RuxTi4 -xO12 were studied for 1 ≤x ≤4 by resistivity, susceptibility, specific-heat measurements, and magnetic-resonance techniques. Our results suggest the existence of a coherent Kondo lattice formed by localized Ru 4 d electrons leading to strongly enhanced effective electron masses. Pure ruthenate (x =4 ) is a heavy-fermion metal characterized by a resistivity proportional to T2 at low temperatures T . By increasing titanium substitution the coherent Fermi-liquid state is disturbed, yielding single-ion Kondo-type properties as in the paradigm 4 f -based heavy-fermion compound CexLa1 -xCu2.05Si2 [M. Ocko et al., Phys. Rev. B 64, 195106 (2001), 10.1103/PhysRevB.64.195106]. In LaCu3RuxTi4 -xO12 the heavy-fermion behavior finally breaks down upon crossing the metal-to-insulator transition close to x =2 .

  5. Kondo Resonance in a Mesoscopic Ring Coupled to a Quantum Dot: Exact Results for the Aharonov-Bohm-Casher Effects

    SciTech Connect

    Eckle, H.-P.; Johannesson, H.; Stafford, C. A.

    2001-07-02

    We study the persistent currents induced by both the Aharonov-Bohm and Aharonov-Casher effects in a one-dimensional mesoscopic ring coupled to a sidebranch quantum dot at Kondo resonance. For privileged values of the Aharonov-Bohm-Casher fluxes, the problem can be mapped onto an integrable model, exactly solvable by a Bethe ansatz. In the case of a pure magnetic Aharonov-Bohm flux, we find that the presence of the quantum dot has no effect on the persistent current. In contrast, the Kondo resonance interferes with the spin-dependent Aharonov-Casher effect to induce a current which, in the strong-coupling limit, is independent of the number of electrons in the ring.

  6. Cubic topological Kondo insulators.

    PubMed

    Alexandrov, Victor; Dzero, Maxim; Coleman, Piers

    2013-11-27

    Current theories of Kondo insulators employ the interaction of conduction electrons with localized Kramers doublets originating from a tetragonal crystalline environment, yet all Kondo insulators are cubic. Here we develop a theory of cubic topological Kondo insulators involving the interaction of Γ(8) spin quartets with a conduction sea. The spin quartets greatly increase the potential for strong topological insulators, entirely eliminating the weak topological phases from the diagram. We show that the relevant topological behavior in cubic Kondo insulators can only reside at the lower symmetry X or M points in the Brillouin zone, leading to three Dirac cones with heavy quasiparticles.

  7. Fano resonance and hybridization gap in the Kondo lattice URu2Si2^*

    NASA Astrophysics Data System (ADS)

    Park, Wan Kyu; Tobash, P. H.; Ronning, F.; Bauer, E. D.; Sarrao, J. L.; Thompson, J. D.; Greene, L. H.

    2012-02-01

    The nature of the `hidden' order transition in URu2Si2 remains puzzling despite intensive research over the past two and half decades. A key question under debate is whether a hybridization gap between the renormalized bands can be identified as the long-sought hidden order parameter. We report on the measurement of a hybridization gap in URu2Si2 employing a spectroscopic technique based on quasiparticle scattering across a ballistic metallic junction [1]. The differential conductance data exhibit an asymmetric double-peak structure, a signature for a Fano resonance in a Kondo lattice [2]. The extracted hybridization gap opens well above the hidden order transition temperature, indicating that it is not the order parameter for the hidden order phase. Our results place constraints on the origin of the hidden order transition in URu2Si2.[4pt] [1] W. K. Park et al., arXiv:1110.5541.[0pt] [2] M. Maltseva, M. Dzero, P. Coleman, PRL 103, 206402 (2009).

  8. Heavy fermion and Kondo lattice behavior in the itinerant ferromagnet CeCrGe3.

    PubMed

    Das, Debarchan; Gruner, T; Pfau, H; Paramanik, U B; Burkhardt, U; Geibel, C; Hossain, Z

    2014-03-12

    Physical properties of polycrystalline CeCrGe3 and LaCrGe3 have been investigated by x-ray absorption spectroscopy, magnetic susceptibility χ(T), isothermal magnetization M(H), electrical resistivity ρ(T), specific heat C(T) and thermoelectric power S(T) measurements. These compounds are found to crystallize in the hexagonal perovskite structure (space group P63/mmc), as previously reported. The ρ(T), χ(T) and C(T) data confirm the bulk ferromagnetic ordering of itinerant Cr moments in LaCrGe3 and CeCrGe3 with TC = 90 K and 70 K respectively. In addition, a weak anomaly is also observed near 3 K in the C(T) data of CeCrGe3. The T dependences of ρ and finite values of Sommerfeld coefficient γ obtained from the specific heat measurements confirm that both the compounds are of metallic character. Further, the T dependence of ρ of CeCrGe3 reflects a Kondo lattice behavior. An enhanced γ of 130 mJ mol(-1) K(-2) together with the Kondo lattice behavior inferred from the ρ(T) establish CeCrGe3 as a moderate heavy fermion compound with a quasi-particle mass renormalization factor of ∼45. PMID:24553355

  9. Resonant behavior of dielectric objects (electrostatic resonances).

    PubMed

    Fredkin, D R; Mayergoyz, I D

    2003-12-19

    Resonant behavior of dielectric objects occurs at certain frequencies for which the object permittivity is negative and the free-space wavelength is large in comparison with the object dimensions. Unique physical features of these resonances are studied and a novel technique for the calculation of resonance values of permittivity, and hence resonance frequencies, is proposed. Scale invariance of resonance frequencies, unusually strong orthogonality properties of resonance modes, and a two-dimensional phenomenon of "twin" spectra are reported. The paper concludes with brief discussions of optical controllability of these resonances in semiconductor nanoparticles and a plausible, electrostatic resonance based, mechanism for nucleation and formation of ball lightning.

  10. Resonant behavior of dielectric objects (electrostatic resonances).

    PubMed

    Fredkin, D R; Mayergoyz, I D

    2003-12-19

    Resonant behavior of dielectric objects occurs at certain frequencies for which the object permittivity is negative and the free-space wavelength is large in comparison with the object dimensions. Unique physical features of these resonances are studied and a novel technique for the calculation of resonance values of permittivity, and hence resonance frequencies, is proposed. Scale invariance of resonance frequencies, unusually strong orthogonality properties of resonance modes, and a two-dimensional phenomenon of "twin" spectra are reported. The paper concludes with brief discussions of optical controllability of these resonances in semiconductor nanoparticles and a plausible, electrostatic resonance based, mechanism for nucleation and formation of ball lightning. PMID:14754117

  11. Theory of Fano Resonances in Graphene: The Kondo effect probed by STM

    SciTech Connect

    Wehling, T.O.

    2010-06-02

    We consider the theory of Kondo effect and Fano factor energy dependence for magnetic impurity (Co) on graphene. We have performed a first principles calculation and find that the two dimensional E{sub 1} representation made of d{sub xz}, d{sub yz} orbitals is likely to be responsible for the hybridization and ultimately Kondo screening for cobalt on graphene. There are few high symmetry sites where magnetic impurity atom can be adsorbed. For the case of Co atom in the middle of hexagon of carbon lattice we find anomalously large Fano q-factor, q {approx} 80 and strongly suppressed coupling to conduction band. This anomaly is a striking example of quantum mechanical interference related to the Berry phase inherent to graphene band structure.

  12. Lattice disorder and size-induced Kondo behavior in CeAl2 andCePt2+x

    SciTech Connect

    Han, S.-W.; Booth, C.H.; Bauer, E.D.; Huang P.H.; Chen, Y.Y.; Lawrence, J.M.

    2006-03-14

    When the particle size of CeAl{sub 2} and CePt{sub 2+x} samples is reduced to the nanometer scale, antiferromagnetism is suppressed and Kondo behavior dominates. We find that the Kondo temperature T{sub K} can either decrease (CeAl{sub 2}) or increase (CePt{sub 2+x}) in the nanoparticles relative to the bulk. Extended x-ray absorption fine-structure data show that the Ce-Al and Ce-Pt environments are significantly distorted in the nanoparticles. While such distortions should strongly affect magnetic and electronic properties, we find they cannot explain the observed changes in T{sub K}. Changes in the conduction density of states or other parameters must, therefore, play a significant role.

  13. First-principles Calculation of the Single Impurity Surface Kondo Resonance

    NASA Astrophysics Data System (ADS)

    Lin, Chiung-Yuan; Castro Neto, Antonio; Jones, Barbara

    2007-03-01

    We have performed first-principles calculation of the surface and bulk wavefunctions of the Cu(111) surface and their hybridization energies to a Co adatom, including the potential scattering from the Co [1]. By analyzing the calculated hybridization energies, we have calculated the Kondo temperature to remarkable accuracy. We find the bulk states dominate the contribution to the Kondo temperature, in agreement with a recent experiment [2]. Furthermore, we also calculate the tunneling conductance of a scanning tunneling microscope on this system and compare our results with recent experiments of Co impurities in the Cu(111) surface. Good quantitative agreement is found at short parallel impurity-tip distances (< 6 angstroms). Our results indicate the need for a new formulation of the problem at larger distances. [1] C.-Y. Lin, A. H. Castro Neto, and B. A. Jones, Phys. Rev. Lett. 97, 156102 (2006). [2] N. Knorr, M. A. Schneider, L. Diekhoner, P. Wahl, and K. Kern, Phys. Rev. Lett. 88, 096804 (2002).

  14. Topological Kondo Insulators

    NASA Astrophysics Data System (ADS)

    Dzero, Maxim; Xia, Jing; Galitski, Victor; Coleman, Piers

    2016-03-01

    This article reviews recent theoretical and experimental work on a new class of topological material -- topological Kondo insulators, which develop through the interplay of strong correlations and spin-orbit interactions. The history of Kondo insulators is reviewed along with the theoretical models used to describe these heavy fermion compounds. The Fu-Kane method of topological classification of insulators is used to show that hybridization between the conduction electrons and localized f electrons in these systems gives rise to interaction-induced topological insulating behavior. Finally, some recent experimental results are discussed, which appear to confirm the theoretical prediction of the topological insulating behavior in samarium hexaboride, where the long-standing puzzle of the residual low-temperature conductivity has been shown to originate from robust surface states.

  15. Kondo physics in the single-electron transistor with ac driving

    SciTech Connect

    Nordlander, Peter; Wingreen, Ned S.; Meir, Yigal; Langreth, David C.

    2000-01-15

    Using a time-dependent Anderson Hamiltonian, a quantum dot with an ac voltage applied to a nearby gate is investigated. A rich dependence of the linear response conductance on the external frequency and driving amplitude is demonstrated. At low frequencies a sufficiently strong ac potential produces sidebands of the Kondo peak in the spectral density of the dot, and a slow, roughly logarithmic decrease in conductance over several decades of frequency. At intermediate frequencies, the conductance of the dot displays an oscillatory behavior due to the appearance of Kondo resonances of the satellites of the dot level. At high frequencies, the conductance of the dot can vary rapidly due to the interplay between photon-assisted tunneling and the Kondo resonance. (c) 2000 The American Physical Society.

  16. The Kondo tip decorated by the Co atom

    NASA Astrophysics Data System (ADS)

    Feng, Wei; Liu, Qin; Lai, Xinchun; Zhao, Aidi

    2016-11-01

    The Kondo effect of single Co adatoms on Ru(0001) is detected with two different kinds of co-decorated tip (Kondo tip) by using low temperature scanning tunneling microscopy and scanning tunneling spectroscopy. We call the relatively separated two magnetic impurities in the tunneling region ‘two Kondo system’ to distinguish it from the ‘two-impurity Kondo system’. We find that the artificially constructed Kondo tips can be generally categorized into two types of Kondo resonances, which have distinct Fano line shapes with quantum interference factor |q| ≫ 1 and |q| ∼ 1, respectively. The tunneling spectra of six constructed two Kondo systems can be well fitted by summing the two Fano resonances of the two subsystems and a linear background. More interestingly, by extracting the amplitudes of the two Fano resonances in the spectra, we find that the electron transmission of such a two Kondo system in the tunneling region is dominated by the quantum interference of the Kondo tip, which is directly related to the geometric configuration of the adsorbed Kondo atom on the tip.

  17. Magnetically induced QCD Kondo effect

    NASA Astrophysics Data System (ADS)

    Ozaki, Sho; Itakura, Kazunori; Kuramoto, Yoshio

    2016-10-01

    The "QCD Kondo effect" stems from the color exchange interaction in QCD with non-Abelian property, and can be realized in a high-density quark matter containing heavy-quark impurities. We propose a novel type of the QCD Kondo effect induced by a strong magnetic field. In addition to the fact that the magnetic field does not affect the color degrees of freedom, two properties caused by the Landau quantization in a strong magnetic field are essential for the "magnetically induced QCD Kondo effect"; (1) dimensional reduction to 1 +1 -dimensions, and (2) finiteness of the density of states for lowest energy quarks. We demonstrate that, in a strong magnetic field B , the scattering amplitude of a massless quark off a heavy quark impurity indeed shows a characteristic behavior of the Kondo effect. The resulting Kondo scale is estimated as ΛK≃√{eqB }αs1 /3exp {-4 π /Ncαslog (4 π /αs)} where αs and Nc are the fine structure constant of strong interaction and the number of colors in QCD, and eq is the electric charge of light quarks.

  18. Non-Fermi liquid behavior and the undersceened Kondo effect in Fe1-yCoySi

    NASA Astrophysics Data System (ADS)

    Wu, Yan; Fulfer, Brad; Chan, Julia; Young, David; Ditusa, John

    2015-03-01

    Mn or Co substitutions into the narrow band-gap insulator FeSi introduce charge carriers, either holes or electrons, accompanied by an equal density of more localized magnetic moments resulting in an interesting insulator-to-metal transition (IMT). Mn doping of FeSi exhibits an IMT where the nascent metal displays intriguing field sensitive non-Fermi-Liquid (NFL) behavior due to the undercompensation of S = 1 impurity moments by the spin-1/2 hole carriers. Here, we present the results of an investigation of Fe1-yCoySi (0 <= y <= 0.1). Our magnetization and susceptibility measurements indicate that for y<0.03 Co-impurities alsointroduce a S = 1 magnetic moment that have a tendency to form singlets whereas for larger ya ferromagnetic interaction that grows with y. We have discovered a NFLbehavior for y<0.03 that evolves into the standard disordered Fermi-liquid form either by applying a magnetic field or by increasing y. The results of specific heat measurements on Fe1-yCoySi,performed to explore the underlying underscreened Kondo mechanism, to investigate its variation with field and composition,and to compare with our Fe1-xMnxSi data will be presented.

  19. Kondo Lattice and Antiferromagnetic Behavior in Quaternary CeTAl4Si2 (T = Rh, Ir) Single Crystals

    NASA Astrophysics Data System (ADS)

    Maurya, Arvind; Kulkarni, Ruta; Thamizhavel, Arumugam; Paudyal, Durga; Dhar, Sudesh Kumar

    2016-03-01

    We have explored in detail the anisotropic magnetic properties of CeRhAl4Si2 and CeIrAl4Si2, which undergo two antiferromagnetic transitions, at TN1 = 12.6 and 15.5 K, followed by a second transition at TN2 = 9.4 and 13.8 K, respectively, with the [001]-axis as the relatively easy axis of magnetization. The electrical resistivity at ambient and applied pressure provides evidence of Kondo interaction in both compounds, further supported by a reduced value of the entropy associated with the magnetic ordering. The Sommerfeld coefficient γ is inferred to be 195.6 and 49.4 mJ/(mol K2) for CeRhAl4Si2 and CeIrAl4Si2, respectively, classifying these materials as moderate heavy-fermion compounds. The crystal electric field energy levels are derived from the peak seen in the Schottky heat capacity. Furthermore, we have also performed electronic structure calculations by using the local spin density approximation + U [LSDA+U] approach, which provide physical insights on the observed magnetic behavior of these two compounds.

  20. Kondo lattice and antiferromagnetic behavior in quaternary CeTAl4Si2 (T = Rh, Ir) single crystals

    DOE PAGES

    Maurya, Arvind; Kulkarni, Ruta; Thamizhavel, Arumugam; Paudyal, Durga; Dhar, Sudesh Kumar

    2016-02-26

    Here, we have explored in detail the anisotropic magnetic properties of CeRhAl4Si2 and CeIrAl4Si2, which undergo two antiferromagnetic transitions, at TN1 = 12.6 and 15.5 K, followed by a second transition at TN2 = 9.4 and 13.8 K, respectively, with the [001]-axis as the relatively easy axis of magnetization. The electrical resistivity at ambient and applied pressure provides evidence of Kondo interaction in both compounds, further supported by a reduced value of the entropy associated with the magnetic ordering. The Sommerfeld coefficient γ is inferred to be 195.6 and 49.4 mJ/(mol K2) for CeRhAl4Si2 and CeIrAl4Si2, respectively, classifying these materialsmore » as moderate heavy-fermion compounds. The crystal electric field energy levels are derived from the peak seen in the Schottky heat capacity. Furthermore, we have also performed electronic structure calculations by using the local spin density approximation + U [LSDA+U] approach, which provide physical insights on the observed magnetic behavior of these two compounds.« less

  1. Kondo peak splitting and Kondo dip induced by a local moment

    PubMed Central

    Niu, Pengbin; Shi, Yun-Long; Sun, Zhu; Nie, Yi-Hang; Luo, Hong-Gang

    2015-01-01

    Many features like spin-orbit coupling, bias and magnetic fields applied, and so on, can strongly influence the Kondo effect. One of the consequences is Kondo peak splitting. However, Kondo peak splitting led by a local moment has not been investigated systematically. In this research we study theoretically electronic transport through a single-level quantum dot exchange coupled to a local magnetic moment in the Kondo regime. We focus on the Kondo peak splitting induced by an anisotropic exchange coupling between the quantum dot and the local moment, which shows rich splitting behavior. We consider the cases of a local moment with S = 1/2 and S = 1. The longitudinal (z-component) coupling plays a role of multivalued magnetic fields and the transverse (x, y-components) coupling lifts the degeneracy of the quantum dot, both of which account for the fine Kondo peak splitting structures. The inter-level or intra-level transition processes are identified in detail. Moreover, we find a Kondo dip at the Fermi level under the proper parameters. The possible experimental observations of these theoretical results should deepen our understanding of Kondo physics. PMID:26658128

  2. The Kondo effect in ferromagnetic atomic contacts.

    PubMed

    Calvo, M Reyes; Fernández-Rossier, Joaquín; Palacios, Juan José; Jacob, David; Natelson, Douglas; Untiedt, Carlos

    2009-04-30

    Iron, cobalt and nickel are archetypal ferromagnetic metals. In bulk, electronic conduction in these materials takes place mainly through the s and p electrons, whereas the magnetic moments are mostly in the narrow d-electron bands, where they tend to align. This general picture may change at the nanoscale because electrons at the surfaces of materials experience interactions that differ from those in the bulk. Here we show direct evidence for such changes: electronic transport in atomic-scale contacts of pure ferromagnets (iron, cobalt and nickel), despite their strong bulk ferromagnetism, unexpectedly reveal Kondo physics, that is, the screening of local magnetic moments by the conduction electrons below a characteristic temperature. The Kondo effect creates a sharp resonance at the Fermi energy, affecting the electrical properties of the system; this appears as a Fano-Kondo resonance in the conductance characteristics as observed in other artificial nanostructures. The study of hundreds of contacts shows material-dependent log-normal distributions of the resonance width that arise naturally from Kondo theory. These resonances broaden and disappear with increasing temperature, also as in standard Kondo systems. Our observations, supported by calculations, imply that coordination changes can significantly modify magnetism at the nanoscale. Therefore, in addition to standard micromagnetic physics, strong electronic correlations along with atomic-scale geometry need to be considered when investigating the magnetic properties of magnetic nanostructures. PMID:19407797

  3. Magnetically Robust Non-Fermi Liquid Behavior in Heavy Fermion Systems with f2-Configuration: Competition between Crystalline-Electric-Field and Kondo-Yosida Singlets

    NASA Astrophysics Data System (ADS)

    Nishiyama, Shinya; Matsuura, Hiroyasu; Miyake, Kazumasa

    2010-10-01

    In f2-based heavy fermion systems with a crystalline-electric-field (CEF) singlet ground state, the non-Fermi liquid (NFL) arises around the quantum critical point (QCP) due to the competition between the CEF singlet and the Kondo-Yosida singlet states. In such a case, the characteristic temperature TF* at which the entropy starts to decrease toward zero is suppressed by the effect of the competition, compared to both energy scales characterizing each singlet state, the lower Kondo temperature (TK2) and the CEF splitting (Δ). We show that in the case of tetragonal symmetry TF* is not affected by the magnetic field up to Hz* which is determined by the distance from the QCP or characteristic energy scales of each singlet states, not by TF* itself. As a result, in the vicinity of QCP, there are parameter regions where the NFL is robust against the magnetic field, at an observable temperature range T > TF*, up to Hz* which is far larger than TF* and less than \\min(TK2,Δ). Our result suggests that such an anomalous NFL behavior can arise also in systems with other CEF symmetry, which might provide us with the basis to understand the anomalous behaviors of UBe13.

  4. Spin versus charge noise from Kondo traps

    NASA Astrophysics Data System (ADS)

    da Silva, Luis G. G. V. Dias; de Sousa, Rogério

    2015-08-01

    Magnetic and charge noise have a common microscopic origin in solid-state devices, as described by a universal electron trap model. In spite of this common origin, magnetic (spin) and charge noise spectral densities display remarkably different behaviors when many-particle correlations are taken into account, leading to the emergence of the Kondo effect. We derive exact frequency sum rules for trap noise and perform numerical renormalization-group calculations to show that while spin noise is a universal function of the Kondo temperature, charge noise remains well described by single-particle theory even when the trap is deep in the Kondo regime. We obtain simple analytical expressions for charge and spin noise that account for Kondo screening in all frequency and temperature regimes, enabling the study of the impact of disorder and the emergence of magnetic 1 /f noise from Kondo traps. We conclude that the difference between charge and spin noise survives even in the presence of disorder, showing that noise can be more manageable in devices that are sensitive to magnetic (rather than charge) fluctuations and that the signature of the Kondo effect can be observed in spin noise spectroscopy experiments.

  5. Evolution of the Coherent State and the Electronic Structure in the Kondo Insulator SmB6

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaohang; Butch, N. P.; Syers, P.; Ziemak, S.; Greene, R. L.; Paglione, J.

    2013-03-01

    As an exemplary Kondo insulator, SmB6 has been studied for several decades; however, direct evidence for the development of the Kondo coherent state and the evolution of the electronic structure in the material has not been obtained due to the rather complicated electronic and thermal transport behavior. Recently, these open questions attracted increasing attention as the emergence of a time-reversal invariant topological surface state in the Kondo insulator has been suggested. Here, we use the quasiparticle tunneling spectroscopy technique to directly investigate the temperature dependence of the electronic states in SmB6. As a signature of the Kondo screening effect in the material, a Fano-like resonance line shape is observed in the tunneling spectroscopy at temperatures below ~ 100 K. We further demonstrate that inter-ion correlation has to be taken into account in order to precisely describe the observed asymmetric tunneling conductance at low temperatures. Our quasiparticle tunneling spectroscopy results also provide important implications for the predicted nontrivial topology in the Kondo insulator. This work is supported by the NSF under Grant No. DMR-1104256.

  6. Behavioral Stochastic Resonance within the Human Brain

    NASA Astrophysics Data System (ADS)

    Kitajo, Keiichi; Nozaki, Daichi; Ward, Lawrence M.; Yamamoto, Yoshiharu

    2003-05-01

    We provide the first evidence that stochastic resonance within the human brain can enhance behavioral responses to weak sensory inputs. We asked subjects to adjust handgrip force to a slowly changing, subthreshold gray level signal presented to their right eye. Behavioral responses were optimized by presenting randomly changing gray levels separately to the left eye. The results indicate that observed behavioral stochastic resonance was mediated by neural activity within the human brain where the information from both eyes converges.

  7. Application of the underscreened Kondo lattice model to neptunium compounds

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simoes, Acirete S.; Iglesias, J. R.; Lacroix, C.; Coqublin, B.

    2012-12-01

    The coexistence of Kondo effect and ferromagnetic order has been observed in many uranium and neptunium compounds such as UTe or Np2PdGa3. This coexistence can be described within the underscreened Anderson lattice model with two f-electrons and S = 1 spins on each site. After performing the Schrieffer-Wolff transformation on this model, we have obtained an effective Hamiltonian with a f-band term in addition to the Kondo interaction for S = 1 spins. The results indicate a coexistence of Kondo effect and ferromagnetic order, with different relative values of the Kondo TK and Curie TC temperatures. We emphasize here especially the case TK < TC where there is a Kondo behavior below TC and a clear decrease of the magnetization below TK. Such a behavior has been observed in the magnetization curves of NpNiSi2 at low temperatures.

  8. Low-temperature (1 K) angle-resolved photoemission investigation of the predicted topological Kondo insulator behavior of SmB6

    NASA Astrophysics Data System (ADS)

    Rader, Oliver; Hlawenka, Peter; Rienks, Emile; Siemensmeyer, Konrad; Weschke, Eugen; Varykhalov, Andrei; Shitsevalova, Natalya; Gabani, Slavomir; Flachbart, Karol

    2015-03-01

    The system SmB6 is known for its unusual resistivity which increases exponentially with decreasing temperature and saturates below 3 K. This has recently been attributed to topological-Kondo-insulator behavior where a topological surface state is created by Sm 4 f - 5 d hybridization and is responsible for the transport. Local-density-approximation + Gutzwiller calculations of the (100) surface predict the appearance of three Dirac cones in the surface Brillouin zone. We perform angle-resolved photoemission at temperatures below 1 K and reveal surface states at Γ and X . Bulk conduction band states near X appear at higher temperature. These findings will be discussed in detail vis-á-vis the theoretical and experimental literature.

  9. From Kondo lattices to Kondo superlattices.

    PubMed

    Shimozawa, Masaaki; Goh, Swee K; Shibauchi, Takasada; Matsuda, Yuji

    2016-07-01

    The realization of new classes of ground states in strongly correlated electron systems continues to be a major issue in condensed matter physics. Heavy fermion materials, whose electronic structure is essentially three-dimensional, are one of the most suitable systems for obtaining novel electronic states because of their intriguing properties associated with many-body effects. Recently, a state-of-the-art molecular beam epitaxy technique was developed to reduce the dimensionality of heavy electron systems by fabricating artificial superlattices that include heavy fermion compounds; this approach can produce a new type of electronic state in two-dimensional (2D) heavy fermion systems. In artificial superlattices of the antiferromagnetic heavy fermion compound CeIn3 and the conventional metal LaIn3, the magnetic order is suppressed by a reduction in the thickness of the CeIn3 layers. In addition, the 2D confinement of heavy fermions leads to enhancement of the effective electron mass and deviation from the standard Fermi liquid electronic properties, which are both associated with the dimensional tuning of quantum criticality. In the superconducting superlattices of the heavy fermion superconductor CeCoIn5 and nonmagnetic metal YbCoIn5, signatures of superconductivity are observed even at the thickness of one unit-cell layer of CeCoIn5. The most remarkable feature of this 2D heavy fermion superconductor is that the thickness reduction of the CeCoIn5 layers changes the temperature and angular dependencies of the upper critical field significantly. This result is attributed to a substantial suppression of the Pauli pair-breaking effect through the local inversion symmetry breaking at the interfaces of CeCoIn5 block layers. The importance of the inversion symmetry breaking in this system has also been supported by site-selective nuclear magnetic resonance spectroscopy, which can resolve spectroscopic information from each layer separately, even within the same CeCoIn5

  10. From Kondo lattices to Kondo superlattices

    NASA Astrophysics Data System (ADS)

    Shimozawa, Masaaki; Goh, Swee K.; Shibauchi, Takasada; Matsuda, Yuji

    2016-07-01

    The realization of new classes of ground states in strongly correlated electron systems continues to be a major issue in condensed matter physics. Heavy fermion materials, whose electronic structure is essentially three-dimensional, are one of the most suitable systems for obtaining novel electronic states because of their intriguing properties associated with many-body effects. Recently, a state-of-the-art molecular beam epitaxy technique was developed to reduce the dimensionality of heavy electron systems by fabricating artificial superlattices that include heavy fermion compounds; this approach can produce a new type of electronic state in two-dimensional (2D) heavy fermion systems. In artificial superlattices of the antiferromagnetic heavy fermion compound CeIn3 and the conventional metal LaIn3, the magnetic order is suppressed by a reduction in the thickness of the CeIn3 layers. In addition, the 2D confinement of heavy fermions leads to enhancement of the effective electron mass and deviation from the standard Fermi liquid electronic properties, which are both associated with the dimensional tuning of quantum criticality. In the superconducting superlattices of the heavy fermion superconductor CeCoIn5 and nonmagnetic metal YbCoIn5, signatures of superconductivity are observed even at the thickness of one unit-cell layer of CeCoIn5. The most remarkable feature of this 2D heavy fermion superconductor is that the thickness reduction of the CeCoIn5 layers changes the temperature and angular dependencies of the upper critical field significantly. This result is attributed to a substantial suppression of the Pauli pair-breaking effect through the local inversion symmetry breaking at the interfaces of CeCoIn5 block layers. The importance of the inversion symmetry breaking in this system has also been supported by site-selective nuclear magnetic resonance spectroscopy, which can resolve spectroscopic information from each layer separately, even within the same CeCoIn5

  11. Voltage Quench Dynamics of a Kondo System.

    PubMed

    Antipov, Andrey E; Dong, Qiaoyuan; Gull, Emanuel

    2016-01-22

    We examine the dynamics of a correlated quantum dot in the mixed valence regime. We perform numerically exact calculations of the current after a quantum quench from equilibrium by rapidly applying a bias voltage in a wide range of initial temperatures. The current exhibits short equilibration times and saturates upon the decrease of temperature at all times, indicating Kondo behavior both in the transient regime and in the steady state. The time-dependent current saturation temperature connects the equilibrium Kondo temperature to a substantially increased value at voltages outside of the linear response. These signatures are directly observable by experiments in the time domain. PMID:26849606

  12. Competing Kondo Effects in Non-Kramers Doublet Systems

    NASA Astrophysics Data System (ADS)

    Kusunose, Hiroaki

    2016-06-01

    In non-Kramers Kondo systems with quadrupolar degrees of freedom, an ordinary magnetic Kondo effect can compete with the quadrupolar Kondo effect. We discuss such competition keeping PrT2Zn20 (T = Ir, Rh) and PrT2Al20 (T = V, Ti) in mind, where the Γ3 non-Kramers crystalline-electric-field (CEF) doublet ground state is realized in a Pr3+ ion with a (4f)2 configuration under cubic symmetry. The quadrupolar Kondo effect can be described by the two-channel Kondo model, which leads to the local non-Fermi-liquid (NFL) ground state, while the magnetic Kondo effect favors the ordinary local Fermi-liquid (FL) ground state. On the basis of the minimal extended two-channel Kondo model including the magnetic Kondo coupling as well, we investigate the competition and resulting thermodynamics, and orbital/magnetic and single-particle excitation spectra by Wilson's numerical renormalization group (NRG) method. There is a first-order transition between the NFL and FL ground states. In addition to these two states, the alternative FL state accompanied by a free magnetic spin appears in the intermediate temperature range, which eventually reaches the true NFL ground state, as a consequence of the stronger competition between the magnetic and quadrupolar Kondo effects. In this peculiar state, the magnetic susceptibility shows a Curie-like behavior, while the orbital fluctuation exhibits the FL behavior. Moreover, the single-particle spectra yield a more singular behavior. Implications to the Pr 1-2-20 systems are briefly discussed.

  13. Kondo force in shuttling devices: dynamical probe for a Kondo cloud.

    PubMed

    Kiselev, M N; Kikoin, K A; Gorelik, L Y; Shekhter, R I

    2013-02-01

    We consider the electromechanical properties of a single-electronic device consisting of a movable quantum dot attached to a vibrating cantilever, forming a tunnel contact with a nonmovable source electrode. We show that the resonance Kondo tunneling of electrons amplifies exponentially the strength of nanoelectromechanical (NEM) coupling in such a device and make the latter insensitive to mesoscopic fluctuations of electronic levels in a nanodot. It is also shown that the study of a Kondo-NEM phenomenon provides additional (as compared with standard conductance measurements in a nonmechanical device) information on retardation effects in the formation of a many-particle cloud accompanying the Kondo tunneling. A possibility for superhigh tunability of mechanical dissipation as well as supersensitive detection of mechanical displacement is demonstrated.

  14. Tunable unconventional Kondo effect on topological insulator surfaces

    NASA Astrophysics Data System (ADS)

    Isaev, L.; Ortiz, G.; Vekhter, I.

    2015-11-01

    We study Kondo physics of a spin-1/2 impurity in electronic matter with strong spin-orbit interaction, which can be realized by depositing magnetic adatoms on the surface of a three-dimensional topological insulator. We show that magnetic properties of topological surface states and the very existence of Kondo screening strongly depend on details of the bulk material, and specifics of surface preparation encoded in time-reversal preserving boundary conditions for electronic wavefunctions. When this tunable Kondo effect occurs, the impurity spin is screened by purely orbital motion of surface electrons. This mechanism gives rise to a transverse magnetic response of the surface metal, and to spin textures that can be used to experimentally probe signatures of a Kondo resonance. Our predictions are particularly relevant for STM measurements in Pb Te -class crystalline topological insulators, but we also discuss implications for other classes of topological materials.

  15. Kondo disorder and non-Fermi-liquid behavior in UCu{sub 5{minus}{ital x}}Pd{sub {ital x}} and CeCu{sub 5.9}Au{sub 0.1}

    SciTech Connect

    Bernal, O.O.; MacLaughlin, D.E.; Amato, A.; Feyerherm, R.; Gygax, F.N.; Schenck, A.; Heffner, R.H.; Le, L.P.; Nieuwenhuys, G.J.; Andraka, B.; Loehneysen, H.v.; Stockert, O.; Ott, H.R.

    1996-11-01

    Muon spin rotation ({mu}SR) has been used to probe non-Fermi-liquid (NFL) behavior in the heavy-fermion alloys UCu{sub 5{minus}{ital x}}Pd{sub {ital x}}, {ital x}=1.0 and 1.5, and CeCu{sub 5.9}Au{sub 0.1}. Zero-field {mu}SR puts an upper bound of {approximately}0.01{mu}{sub {ital B}}/{ital U} atom on any static magnetism in UCu{sub 5{minus}{ital x}}Pd{sub {ital x}}, which is too weak to affect the transverse-field {mu}SR linewidth or to give rise to NFL behavior. In agreement with NMR results, {mu}SR spectra in transverse fields suggest that a broad distribution of Kondo temperatures ({open_quote}{open_quote}Kondo disorder{close_quote}{close_quote}) is important in UCu{sub 5{minus}{ital x}}Pd{sub {ital x}}. NFL anomalies at temperature {ital T} then arise from {open_quote}{open_quote}free{close_quote}{close_quote} spins for which {ital T}{sub {ital K}}{lt}{ital T}. Comparison of {mu}SR and NMR linewidths also indicates short-range spatial correlation of the Kondo disorder in UCu{sub 5{minus}{ital x}}Pd{sub {ital x}}, in agreement with the local character of the dynamic susceptibility inferred from neutron scattering experiments. In CeCu{sub 5.9}Au{sub 0.1} the data suggest significant Kondo disorder only if the spatial correlation is long ranged, which is not indicated by other properties of this alloy. {copyright} {ital 1996 The American Physical Society.}

  16. Schwinger boson approach to the fully screened Kondo model.

    PubMed

    Rech, J; Coleman, P; Zarand, G; Parcollet, O

    2006-01-13

    We apply the Schwinger boson scheme to the fully screened Kondo model and generalize the method to include antiferromagnetic interactions between ions. Our approach captures the Kondo crossover from local moment behavior to a Fermi liquid with a nontrivial Wilson ratio. When applied to the two-impurity model, the mean-field theory describes the "Varma-Jones" quantum phase transition between a valence bond state and a heavy Fermi liquid.

  17. Competition between Kondo Screening and Quantum Hall Edge Reconstruction.

    PubMed

    Heine, A W; Tutuc, D; Zwicknagl, G; Haug, R J

    2016-03-01

    We report on a Kondo correlated quantum dot connected to two-dimensional leads where we demonstrate the renormalization of the g factor in the pure Zeeman case. i.e., for magnetic fields parallel to the plane of the quantum dot. For the same system, we study the influence of orbital effects by investigating the quantum Hall regime; i.e., a perpendicular magnetic field is applied. In this case an unusual behavior of the suppression of the Kondo effect and of the split zero-bias anomaly is observed. The splitting decreases with magnetic field and shows discontinuous changes that are attributed to the intricate interplay between Kondo screening and the quantum Hall edge structure originating from electrostatic screening. This edge structure, made up of compressible and incompressible stripes, strongly affects the Kondo temperature of the quantum dot and thereby influences the renormalized g factor. PMID:26991192

  18. Competition between Kondo Screening and Quantum Hall Edge Reconstruction

    NASA Astrophysics Data System (ADS)

    Heine, A. W.; Tutuc, D.; Zwicknagl, G.; Haug, R. J.

    2016-03-01

    We report on a Kondo correlated quantum dot connected to two-dimensional leads where we demonstrate the renormalization of the g factor in the pure Zeeman case. i.e., for magnetic fields parallel to the plane of the quantum dot. For the same system, we study the influence of orbital effects by investigating the quantum Hall regime; i.e., a perpendicular magnetic field is applied. In this case an unusual behavior of the suppression of the Kondo effect and of the split zero-bias anomaly is observed. The splitting decreases with magnetic field and shows discontinuous changes that are attributed to the intricate interplay between Kondo screening and the quantum Hall edge structure originating from electrostatic screening. This edge structure, made up of compressible and incompressible stripes, strongly affects the Kondo temperature of the quantum dot and thereby influences the renormalized g factor.

  19. Laser-Induced Kondo Effect in Ultracold Alkaline-Earth Fermions.

    PubMed

    Nakagawa, Masaya; Kawakami, Norio

    2015-10-16

    We demonstrate that laser excitations can coherently induce a novel Kondo effect in ultracold atoms in optical lattices. Using a model of alkaline-earth fermions with two orbitals, it is shown that the optically coupled two internal states are dynamically entangled to form the Kondo-singlet state, overcoming the heating effect due to the irradiation. Furthermore, a lack of SU(N) symmetry in the optical coupling provides a peculiar feature in the Kondo effect, which results in spin-selective renormalization of effective masses. We also discuss the effects of interorbital exchange interactions, and reveal that they induce novel crossover or reentrant behavior of the Kondo effect owing to control of the coupling anisotropy. The laser-induced Kondo effect is highly controllable by tuning the laser strength and the frequency, and thus offers a versatile platform to study the Kondo physics using ultracold atoms.

  20. Panel resonant behavior of wind turbine blades.

    SciTech Connect

    Paquette, Joshua A.; Griffith, Daniel Todd

    2010-03-01

    The principal design drivers in the certification of wind turbine blades are ultimate strength, fatigue resistance, adequate tip-tower clearance, and buckling resistance. Buckling resistance is typically strongly correlated to both ultimate strength and fatigue resistance. A composite shell with spar caps forms the airfoil shape of a blade and reinforcing shear webs are placed inside the blade to stiffen the blade in the flap-wise direction. The spar caps are dimensioned and the shear webs are placed so as to add stiffness to unsupported panel regions and reduce their length. The panels are not the major flap-wise load carrying element of a blade; however, they must be designed carefully to avoid buckling while minimizing blade weight. Typically, buckling resistance is evaluated by consideration of the load-deflection behavior of a blade using finite element analysis (FEA) or full-scale static testing of blades under a simulated extreme loading condition. The focus of this paper is on the use of experimental modal analysis to measure localized resonances of the blade panels. It can be shown that the resonant behavior of these panels can also provide a means to evaluate buckling resistance by means of analytical or experimental modal analysis. Further, panel resonances have use in structural health monitoring by observing changes in modal parameters associated with panel resonances, and use in improving panel laminate model parameters by correlation with test data. In recent modal testing of wind turbine blades, a set of panel modes were measured. This paper will report on the findings of these tests and accompanying numerical and analytical modeling efforts aimed at investigating the potential uses of panel resonances for blade evaluation, health monitoring, and design.

  1. Measurement of Valley Kondo Effect in a Si/SiGe Quantum Dot

    NASA Astrophysics Data System (ADS)

    Yuan, Mingyun; Yang, Zhen; Tang, Chunyang; Rimberg, A. J.; Joynt, R.; Savage, D. E.; Lagally, M. G.; Eriksson, M. A.

    2013-03-01

    The Kondo effect in Si/SiGe QDs can be enriched by the valley degree of freedom in Si. We have observed resonances showing temperature dependence characteristic of the Kondo effect in two consecutive Coulomb diamonds. These resonances exhibit unusual magnetic field dependence that we interpret as arising from Kondo screening of the valley degree of freedom. In one diamond two Kondo peaks due to screening of the valley index exist at zero magnetic field, revealing a zero-field valley splitting of Δ ~ 0.28 meV. In a non-zero magnetic field the peaks broaden and coalesce due to Zeeman splitting. In the other diamond, a single resonance at zero bias persists without Zeeman splitting for non-zero magnetic field, a phenomenon characteristic of valley non-conservation in tunneling. This research is supported by the NSA and ARO.

  2. Surface Kondo Impurities in the Slave-Boson Approach

    NASA Astrophysics Data System (ADS)

    Anda, Enrique; Vernek, Edson

    2005-03-01

    Transport properties of magnetic impurities on surfaces have captured a great deal of attention lately. Atom manipulation and topographic imaging techniques using scanning tunneling microscope have confirmed some theoretical predictions on Kondo physics and at the same time revealed other interesting behavior in these systems. For example, experiments have reported unexpectedly high Kondo temperatures for multi-impurity and molecular structures on metallic surfaces. Motivated by these experimental results we apply slave boson techniques for finite Coulomb interaction (finite U) to study the transport properties of magnetic impurities on a metallic surface in the Kondo regime. We report here on our studies of the role of fluctuations on the slave boson number for the case of one impurity on metallic surfaces. We compare our results to other theoretical approaches and to experimental results. Supported by CAPES-Brazil and NSF-IMC and NSF-NIRT.

  3. Simple Description of the Two-Channel Kondo Problem

    NASA Astrophysics Data System (ADS)

    Coleman, Piers

    1996-03-01

    The physics of the two channel Kondo model provides an example of a new universality class of non-Fermi liquid behavior. Its spin physics provides one of the few concrete examples of true marginal Fermi liquid behavior. Two channel Kondo physics may also provide one of basic engines for non Fermi liquid behavior in heavy fermion systems. For these reasons, a simple description of the underlying physics in this model is highly desirable. Conventionally, this model had yielded only to the most sophisticated and specialized mathematical techniques. I shall explain (P.Coleman, L. Ioffe and A. M. Tsvelik, Phys. Rev. B), 52, 6611 (1995). (P. Coleman and A. Schofield, Phys. Rev. Lett), 75, 2184, (1995) how we have been able to circumvent the problems encountered by earlier attempts to develop a simple picture by reformulating the two-channel Kondo model to explicitly remove the unscattered charge degrees of freedom from the outset. This procedure moves the non-Fermi liquid fixed point to infinite coupling where simple back-of-the envelope methods reveals the secret workings of its marginal Fermi liquid fixed point. I shall carefully explain how marginal spin-physics of the two-channel Kondo model results from the formation of a neutral three-body bound state at the Fermi energy. This new physics may prove to be very important as a guide to our general understanding of marginal Fermi liquid behavior.

  4. Spin polarization of the split Kondo state.

    PubMed

    von Bergmann, Kirsten; Ternes, Markus; Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

    2015-02-20

    Spin-resolved scanning tunneling microscopy is employed to quantitatively determine the spin polarization of the magnetic field-split Kondo state. Tunneling conductance spectra of a Kondo-screened magnetic atom are evaluated within a simple model taking into account inelastic tunneling due to spin excitations and two Kondo peaks positioned symmetrically around the Fermi energy. We fit the spin state of the Kondo-screened atom with a spin Hamiltonian independent of the Kondo effect and account for Zeeman splitting of the Kondo peak in the magnetic field. We find that the width and the height of the Kondo peaks scales with the Zeeman energy. Our observations are consistent with full spin polarization of the Kondo peaks, i.e., a majority spin peak below the Fermi energy and a minority spin peak above. PMID:25763966

  5. A Maximally Supersymmetric Kondo Model

    SciTech Connect

    Harrison, Sarah; Kachru, Shamit; Torroba, Gonzalo; /Stanford U., Phys. Dept. /SLAC

    2012-02-17

    We study the maximally supersymmetric Kondo model obtained by adding a fermionic impurity to N = 4 supersymmetric Yang-Mills theory. While the original Kondo problem describes a defect interacting with a free Fermi liquid of itinerant electrons, here the ambient theory is an interacting CFT, and this introduces qualitatively new features into the system. The model arises in string theory by considering the intersection of a stack of M D5-branes with a stack of N D3-branes, at a point in the D3 worldvolume. We analyze the theory holographically, and propose a dictionary between the Kondo problem and antisymmetric Wilson loops in N = 4 SYM. We perform an explicit calculation of the D5 fluctuations in the D3 geometry and determine the spectrum of defect operators. This establishes the stability of the Kondo fixed point together with its basic thermodynamic properties. Known supergravity solutions for Wilson loops allow us to go beyond the probe approximation: the D5s disappear and are replaced by three-form flux piercing a new topologically non-trivial S3 in the corrected geometry. This describes the Kondo model in terms of a geometric transition. A dual matrix model reflects the basic properties of the corrected gravity solution in its eigenvalue distribution.

  6. Proposal to directly observe the Kondo effect through enhanced photoinduced scattering of cold fermionic and bosonic atoms

    NASA Astrophysics Data System (ADS)

    Sundar, Bhuvanesh; Mueller, Erich J.

    2016-02-01

    We propose an experimental protocol to directly observe the Kondo effect by scattering ultracold atoms. We propose using an optical Feshbach resonance to engineer Kondo-type spin-dependent interactions in a system with ultracold 6Li and 87Rb gases. We calculate the momentum transferred from the 87Rb gas to the 6Li gas in a scattering experiment and show that it has a logarithmically enhanced temperature dependence, characteristic of the Kondo effect, and analogous to the resistivity of alloys with magnetic impurities. Experimentally detecting this enhancement will give a different perspective on the Kondo effect, and allow us to explore a rich variety of problems such as the Kondo lattice problem and heavy-fermion systems.

  7. Kondo effect in a quantum dot side-coupled to a topological superconductor

    NASA Astrophysics Data System (ADS)

    Lee, Minchul; Lim, Jong Soo; López, Rosa

    2013-06-01

    We investigate the dynamical and transport features of a Kondo dot side coupled to a topological superconductor (TS). The Majorana fermion states (MFSs) formed at the ends of the TS are found to be able to alter the Kondo physics profoundly: For an infinitely long wire where the MFSs do not overlap (ɛm=0) a finite dot-MFS coupling (Γm) reduces the unitary-limit value of the linear conductance by exactly a factor 3/4 in the weak-coupling regime (ΓmKondo temperature. In the strong-coupling regime (Γm>TK), on the other hand, the spin-split Kondo resonance takes place due to the MFS-induced Zeeman splitting, which is a genuine many-body effect of the strong Coulomb interaction and the topological superconductivity. We find that the original Kondo resonance is fully restored once the MFSs are strongly hybridized (ɛm>Γm). This unusual interaction between the Kondo effect and the MFS can thus serve to detect the Majorana fermions unambiguously and quantify the degree of overlap between the MFSs in the TS.

  8. Magnetically robust non-fermi liquid behavior due to the competition between crystalline-electric field singlet and Kondo-Yosida singlet in f2-based heavy fermion systems

    NASA Astrophysics Data System (ADS)

    Nishiyama, Shinya; Matsuura, Hiroyasu; Miyake, Kazumasa

    2011-01-01

    In f2-based heavy fermion systems with a tetragonal symmetry, we investigate the magnetic field dependence of a non-fermi liquid (NFL) which arises related to the quantum critical point (QCP) due to the competition between the crystalline-electric field (CEF) singlet and the Kondo-Yosida singlet states. On the basis of the Wilson numerical renormalization group method, we find that the magnetic field less than a characteristic magnetic field Hz* does not affect the characteristic temperature TF* at which the specific heat takes a maximum value. Since such Hz* increases as the deviation from the QCP increases, slightly off the QCP, there are parameter regions where NFL behaviors are robust at an observable temperature range T > TF*against a magnetic field of up to Hz* which is far larger than TF*. Our result suggests that such robust NFL behaviors can arise also in systems with other CEF symmetries; e.g., magnetically robust NFL behaviors observed in UBe13 may be understood on this basis.

  9. Controlling orbital-selective Kondo effects in a single molecule through coordination chemistry

    SciTech Connect

    Tsukahara, Noriyuki; Kawai, Maki; Takagi, Noriaki; Minamitani, Emi; Kim, Yousoo

    2014-08-07

    Iron(II) phthalocyanine (FePc) molecule causes novel Kondo effects derived from the unique electronic structure of multi-spins and multi-orbitals when attached to Au(111). Two unpaired electrons in the d{sub z}{sup 2} and the degenerate dπ orbitals are screened stepwise, resulting in spin and spin+orbital Kondo effects, respectively. We investigated the impact on the Kondo effects of the coordination of CO and NO molecules to the Fe{sup 2+} ion as chemical stimuli by using scanning tunneling microscopy (STM) and density functional theory calculations. The impacts of the two diatomic molecules are different from each other as a result of the different electronic configurations. The coordination of CO converts the spin state from triplet to singlet, and then the Kondo effects completely disappear. In contrast, an unpaired electron survives in the molecular orbital composed of Fe d{sub z}{sup 2} and NO 5σ and 2π* orbitals for the coordination of NO, causing a sharp Kondo resonance. The isotropic magnetic response of the peak indicates the origin is the spin Kondo effect. The diatomic molecules attached to the Fe{sup 2+} ion were easily detached by applying a pulsed voltage at the STM junction. These results demonstrate that the single molecule chemistry enables us to switch and control the spin and the many-body quantum states reversibly.

  10. Maximized orbital and spin Kondo effect in a single electron box

    NASA Astrophysics Data System (ADS)

    Le Hur, Karyn

    2004-03-01

    We investigate the charge fluctuations of a metallic grain (large dot) coupled to a bank of electrons via a smaller dot in the Kondo regime. The most interesting aspect of this problem resides in the interplay between "spin" Kondo physics stemming from the screening of the spin of the small dot, and "orbital" Kondo effect emerging when charging states of the grain with (charge) Q=0 and Q=e are almost degenerate. We emphasize that for symmetric or slightly asymmetric tunneling barriers, the strong entanglement of charge and spin flips results in a fascinating Kondo liquid with SU(4) symmetry. This considerably smears out the Coulomb staircase behavior of the grain's charge already in the weak tunneling regime. Different crossovers and experimental consequences will be addressed. Refs: K. Le Hur and P. Simon, PRB 67, R201308 (2003); K. Le Hur, P. Simon, and L. Borda, cond-mat/0306186 (to appear in PRB)

  11. Emergence of a Fermionic Finite-Temperature Critical Point in a Kondo Lattice.

    PubMed

    Chou, Po-Hao; Zhai, Liang-Jun; Chung, Chung-Hou; Mou, Chung-Yu; Lee, Ting-Kuo

    2016-04-29

    The underlying Dirac point is central to the profound physics manifested in a wide class of materials. However, it is often difficult to drive a system with Dirac points across the massless fermionic critical point. Here by exploiting screening of local moments under spin-orbit interactions in a Kondo lattice, we show that below the Kondo temperature, the Kondo lattice undergoes a topological transition from a strong topological insulator to a weak topological insulator at a finite temperature T_{D}. At T_{D}, massless Dirac points emerge and the Kondo lattice becomes a Dirac semimetal. Our analysis indicates that the emergent relativistic symmetry dictates nontrivial thermal responses over large parameter and temperature regimes. In particular, it yields critical scaling behaviors both in magnetic and transport responses near T_{D}.

  12. Emergence of a Fermionic Finite-Temperature Critical Point in a Kondo Lattice

    NASA Astrophysics Data System (ADS)

    Chou, Po-Hao; Zhai, Liang-Jun; Chung, Chung-Hou; Mou, Chung-Yu; Lee, Ting-Kuo

    2016-04-01

    The underlying Dirac point is central to the profound physics manifested in a wide class of materials. However, it is often difficult to drive a system with Dirac points across the massless fermionic critical point. Here by exploiting screening of local moments under spin-orbit interactions in a Kondo lattice, we show that below the Kondo temperature, the Kondo lattice undergoes a topological transition from a strong topological insulator to a weak topological insulator at a finite temperature TD. At TD, massless Dirac points emerge and the Kondo lattice becomes a Dirac semimetal. Our analysis indicates that the emergent relativistic symmetry dictates nontrivial thermal responses over large parameter and temperature regimes. In particular, it yields critical scaling behaviors both in magnetic and transport responses near TD.

  13. Multiorbital Kondo physics of Co in Cu hosts

    NASA Astrophysics Data System (ADS)

    Surer, Brigitte; Troyer, Matthias; Werner, Philipp; Wehling, Tim O.; Läuchli, Andreas M.; Wilhelm, Aljoscha; Lichtenstein, Alexander I.

    2012-02-01

    We investigate the electronic structure of cobalt atoms on a copper surface and in a copper host by combining density-functional calculations with a numerically exact continuous-time quantum Monte Carlo treatment of the five-orbital impurity problem. In both cases we find low energy resonances in the density of states of all five Co d orbitals. The corresponding self-energies indicate the formation of a Fermi liquid state at low temperatures. Our calculations yield the characteristic energy scale—the Kondo temperature—for both systems in good agreement with experiments. We quantify the charge fluctuations in both geometries and suggest that Co in Cu must be described by an Anderson impurity model rather than by a model assuming frozen impurity valency at low energies. We show that fluctuations of the orbital degrees of freedom are crucial for explaining the Kondo temperatures obtained in our calculations and measured in experiments.

  14. Multi-orbital Kondo physics of Co in Cu hosts

    NASA Astrophysics Data System (ADS)

    Lichtenstein, Alexander; Wehling, Tim Oliver; Wilhelm, Aljoscha; Surer, Brigitte; Troyer, Matthias; Werner, Philipp; Läuchli, Andreas

    2012-02-01

    We investigate the electronic structure of cobalt atoms on a copper surface and in a copper host by combining density functional calculations with a numerically exact continuous-time quantum Monte Carlo treatment of the five-orbital impurity problem. In both cases we find low energy resonances in the density of states of all five Co d-orbitals. The corresponding self-energies indicate the formation of a Fermi liquid state at low temperatures. Our calculations yield the characteristic energy scale -- the Kondo temperature -- for both systems in good agreement with experiments. We quantify the charge fluctuations in both geometries and suggest that Co in Cu must be described by an Anderson impurity model rather than by a model assuming frozen impurity valency at low energies. We show that fluctuations of the orbital degrees of freedom are crucial for explaining the Kondo temperatures obtained in our calculations and measured in experiments.

  15. Antiferromagnetism and Kondo screening on a honeycomb lattice

    NASA Astrophysics Data System (ADS)

    Lin, Heng-Fu; Hong-Shuai, Tao; Guo, Wen-Xiang; Liu, Wu-Ming

    2015-05-01

    Magnetic adatoms in the honeycomb lattice have received tremendous attention due to the interplay between Ruderman-Kittel-Kasuya-Yosida interaction and Kondo coupling leading to very rich physics. Here we study the competition between the antiferromagnetism and Kondo screening of local moments by the conduction electrons on the honeycomb lattice using the determinant quantum Monte Carlo method. While changing the interband hybridization V, we systematically investigate the antiferromagnetic-order state and the Kondo singlet state transition, which is characterized by the behavior of the local moment, antiferromagnetic structure factor, and the short range spin-spin correlation. The evolution of the single particle spectrum are also calculated as a function of hybridization V, we find that the system presents a small gap in the antiferromagnetic-order region and a large gap in the Kondo singlet region in the Fermi level. We also find that the localized and itinerant electrons coupling leads to the midgap states in the conduction band in the Fermi level at very small V. Moreover, the formation of antiferromagnetic order and Kondo singlet are studied as on-site interaction U or temperature T increasing, we have derived the phase diagrams at on-site interaction U (or temperature T) and hybridization V plane. Project supported by the National Key Basic Research Special Foundation of China (Grants Nos. 2011CB921502 and 2012CB821305), the National Natural Science Foundation of China (Grants Nos. 61227902, 61378017, and 11434015), the State Key Laboratory for Quantum Optics and Quantum Optical Devices, China (Grant No. KF201403).

  16. Resonance behavior of atomic and molecular photoionization amplitudes

    SciTech Connect

    Cherepkov, N. A.; Kuznetsov, V. V.; Semenov, S. K.

    2007-07-15

    The behavior of the partial photoionization amplitudes with a given orbital angular momentum l in the complex plane in resonances is studied. In the autoionization resonances the trajectory of the amplitude in the complex plane corresponds to a circle. With increasing photoelectron energy the amplitude moves about a circle in the counterclockwise direction. The new expressions for the partial amplitudes in the resonance are proposed which are similar to the Fano form but contain the 'partial' profile parameters which are connected with the Fano parameter q by a simple relation. In the giant dipole resonances the amplitudes in the complex plane also move about a circle in the counterclockwise direction provided the Coulomb phase is excluded from the amplitude. In the correlational resonances created by channel interactions with the giant dipole resonance the trajectories of the amplitudes acquire a loop about which the amplitudes move in the counterclockwise direction. Very similar behavior of partial photoionization amplitudes in the complex plane is demonstrated also for the dipole transitions from the K shells of the N{sub 2} molecule in the {sigma}* shape resonance.

  17. Magnetic Field Effect on Crossover Temperature from Non-Fermi Liquid to Fermi Liquid Behavior in f2-Impurity Systems with Crystalline-Electric-Field Singlet State Competing with Kondo--Yosida Singlet State

    NASA Astrophysics Data System (ADS)

    Nishiyama, Shinya; Miyake, Kazumasa

    2011-12-01

    We investigate the magnetic field dependence of the physical properties of f2-configuration systems with a crystalline-electric field (CEF) singlet ground state, which gives rise to a non-Fermi liquid (NFL) fixed point due to the competition between the Kondo--Yosida singlet and CEF singlet states. On the basis of the numerical renormalization group method, we find that the magnetic field breaks this NFL fixed point via two mechanisms: one causing the polarization of f-electrons and the other giving the ``channel'' anisotropy. These two mechanisms induce a difference in the magnetic field dependence of the characteristic temperature TF*(H), the crossover temperature from NFL to Fermi-liquid behavior. While the polarization of f-electrons gives TF*(H) \\propto Hx (x ≃ 2.0), the ``channel'' anisotropy gives the H-independent TF*(H). These two mechanisms cross over continuously at approximately the crossover magnetic field Hc, where an anomalous H-dependence of TF*(H) appears. Such TF*(H) well reproduces the NFL behaviors observed in Th1-xUxRu2Si2. We also find that the H-dependence of the resistivity and the magnetic susceptibility are in good agreement with the experimental results of this material. These results suggest that the NFL behaviors observed in Th1-xUxRu2Si2 can be understood if this material is located in the CEF singlet side near the critical phase boundary between the two singlet states.

  18. Macroscopic quantum entanglement of a Kondo cloud at finite temperature.

    PubMed

    Lee, S-S B; Park, Jinhong; Sim, H-S

    2015-02-01

    We propose a variational approach for computing the macroscopic entanglement in a many-body mixed state, based on entanglement witness operators, and compute the entanglement of formation (EoF), a mixed-state generalization of the entanglement entropy, in single- and two-channel Kondo systems at finite temperature. The thermal suppression of the EoF obeys power-law scaling at low temperature. The scaling exponent is halved from the single- to the two-channel system, which is attributed, using a bosonization method, to the non-Fermi liquid behavior of a Majorana fermion, a "half" of a complex fermion, emerging in the two-channel system. Moreover, the EoF characterizes the size and power-law tail of the Kondo screening cloud of the single-channel system.

  19. Conductance fingerprint of Majorana fermions in the topological Kondo effect

    NASA Astrophysics Data System (ADS)

    Galpin, Martin R.; Mitchell, Andrew K.; Temaismithi, Jesada; Logan, David E.; Béri, Benjamin; Cooper, Nigel R.

    2014-01-01

    We consider an interacting nanowire/superconductor heterostructure attached to metallic leads. The device is described by an unusual low-energy model involving spin-1 conduction electrons coupled to a nonlocal spin-1/2 Kondo impurity built from Majorana fermions. The topological origin of the resulting Kondo effect is manifest in distinctive non-Fermi-liquid (NFL) behavior, and the existence of Majorana fermions in the device is demonstrated unambiguously by distinctive conductance line shapes. We study the physics of the model in detail, using the numerical renormalization group, perturbative scaling, and Abelian bosonization. In particular, we calculate the full scaling curves for the differential conductance in ac and dc fields, onto which experimental data should collapse. Scattering t matrices and thermodynamic quantities are also calculated, recovering asymptotes from conformal field theory. We show that the NFL physics is robust to asymmetric Majorana-lead couplings, and here we uncover a duality between strong and weak coupling. The NFL behavior is understood physically in terms of competing Kondo effects. The resulting frustration is relieved by inter-Majorana coupling which generates a second crossover to a regular Fermi liquid.

  20. Resonance Angle Nodding Behavior for Planet Pairs Near Mean Motion Resonance

    NASA Astrophysics Data System (ADS)

    Ketchum, Jake; Adams, F. C.; Bloch, A. M.

    2012-05-01

    Motivated by the large number of extrasolar planetary systems that are near mean motion resonances, this paper explores a related type of dynamical behavior known as “nodding”. Here, the resonance angle of a planetary system executes libration (oscillatory motion) for several cycles, circulates for one or more cycles, and then enters once again into libration. This type of complicated dynamics can affect our interpretation of observed planetary systems that are in or near mean motion resonance. This work shows that planetary systems in mean motion resonance can exhibit nodding behavior, and outlines the portion of parameter space where it occurs. This problem is addressed using both full numerical integrations of the planetary systems and via model equations obtained through expansions of the disturbing function. In the latter approach, we identify the relevant terms that allow for nodding. The two approaches are in agreement, and show that nodding often occurs when a small body is in an external mean motion resonance with a larger planet. As a result, this phenomena can be important for interpreting observations of transit timing variations, where the existence of smaller bodies is inferred through their effects on larger, observed transiting planets.

  1. Broken SU(4) symmetry in a Kondo-correlated carbon nanotube

    NASA Astrophysics Data System (ADS)

    Schmid, Daniel R.; Smirnov, Sergey; Margańska, Magdalena; Dirnaichner, Alois; Stiller, Peter L.; Grifoni, Milena; Hüttel, Andreas K.; Strunk, Christoph

    2015-04-01

    Understanding the interplay between many-body phenomena and nonequilibrium in systems with entangled spin and orbital degrees of freedom is a central objective in nanoelectronics. We demonstrate that the combination of Coulomb interaction, spin-orbit coupling, and valley mixing results in a particular selection of the inelastic virtual processes contributing to the Kondo resonance in carbon nanotubes at low temperatures. This effect is dictated by conjugation properties of the underlying carbon nanotube spectrum at zero and finite magnetic field. Our measurements on a clean carbon nanotube are complemented by calculations based on a field-theoretical Keldysh approach to the nonequilibrium Kondo problem which well reproduces the rich experimental observations in Kondo transport.

  2. Quantum dots with even number of electrons: kondo effect in a finite magnetic field

    PubMed

    Pustilnik; Avishai; Kikoin

    2000-02-21

    We show that the Kondo effect can be induced by an external magnetic field in quantum dots with an even number of electrons. If the Zeeman energy B is close to the single-particle level spacing Delta in the dot, the scattering of the conduction electrons from the dot is dominated by an anisotropic exchange interaction. A Kondo resonance then occurs despite the fact that B exceeds by far the Kondo temperature T(K). As a result, at low temperatures T

  3. Universality of the Kondo effect in quantum dots with ferromagnetic leads.

    PubMed

    Gaass, M; Hüttel, A K; Kang, K; Weymann, I; von Delft, J; Strunk, Ch

    2011-10-21

    We investigate quantum dots in clean single-wall carbon nanotubes with ferromagnetic PdNi-leads in the Kondo regime. Most of the Kondo resonances exhibit a splitting, which depends on the tunnel coupling to the leads and an external magnetic field B, but only weakly on the gate voltage. Using numerical renormalization group calculations, we demonstrate that all salient features of the data can be understood using a simple model for the magnetic properties of the leads. The magnetoconductance at zero bias and low temperature depends in a universal way on gμ(B)(B-B(c))/k(B)T(K), where T(K) is the Kondo temperature and B(c) the external field compensating the splitting. PMID:22107560

  4. Kondo interactions from band reconstruction in YbInCu4

    DOE PAGES

    Jarrige, I.; Kotani, A.; Yamaoka, H.; Tsujii, N.; Ishii, K.; Upton, M.; Casa, D.; Kim, J.; Gog, T.; Hancock, J. N.

    2015-03-27

    We combine resonant inelastic X-ray scattering (RIXS) and model calculations in the Kondo lattice compound YbInCu₄, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T≃42 K. In this study, the bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasi-gap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system.

  5. Kondo interactions from band reconstruction in YbInCu(4).

    PubMed

    Jarrige, I; Kotani, A; Yamaoka, H; Tsujii, N; Ishii, K; Upton, M; Casa, D; Kim, J; Gog, T; Hancock, J N

    2015-03-27

    We combine resonant inelastic x-ray scattering and model calculations in the Kondo lattice compound YbInCu_{4}, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T≃42  K. The bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasigap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system. PMID:25860761

  6. Motor resonance evoked by observation of subtle nonverbal behavior.

    PubMed

    van Ulzen, Niek R; Fiorio, Mirta; Cesari, Paola

    2013-01-01

    This study was designed to combine two, otherwise separated, fields of research regarding motor resonance and mimicry by adopting a naturalistic mimicry paradigm while probing motor resonance with transcranial magnetic stimulation (TMS). At stake was whether the motor system resonates instantaneously with unobtrusive nonverbal behavior of another person. We measured excitability in the left and right hand while participants viewed sequences of video clips and static images. In the video clips an actor performed several clerical tasks, while either inconspicuously touching his face (face-touching (FT) condition) or not (no face-touching (NFT) condition). We found that excitability was higher in the FT condition than in the NFT and baseline conditions. Furthermore, our data showed a general heightened excitability in the left motor cortex relative to the right. Taken together, the results suggest that observed hand-face gestures--even though outside the primary focus of attention and occurring inconspicuously throughout an ongoing action setting--can cause instantaneous resonant activity in the observer's motor system. It thus supports the idea of motor resonance involvement in mimicry and demonstrates that this can be studied using a naturalistic mimicry paradigm. PMID:23758553

  7. Motor resonance evoked by observation of subtle nonverbal behavior.

    PubMed

    van Ulzen, Niek R; Fiorio, Mirta; Cesari, Paola

    2013-01-01

    This study was designed to combine two, otherwise separated, fields of research regarding motor resonance and mimicry by adopting a naturalistic mimicry paradigm while probing motor resonance with transcranial magnetic stimulation (TMS). At stake was whether the motor system resonates instantaneously with unobtrusive nonverbal behavior of another person. We measured excitability in the left and right hand while participants viewed sequences of video clips and static images. In the video clips an actor performed several clerical tasks, while either inconspicuously touching his face (face-touching (FT) condition) or not (no face-touching (NFT) condition). We found that excitability was higher in the FT condition than in the NFT and baseline conditions. Furthermore, our data showed a general heightened excitability in the left motor cortex relative to the right. Taken together, the results suggest that observed hand-face gestures--even though outside the primary focus of attention and occurring inconspicuously throughout an ongoing action setting--can cause instantaneous resonant activity in the observer's motor system. It thus supports the idea of motor resonance involvement in mimicry and demonstrates that this can be studied using a naturalistic mimicry paradigm.

  8. Influence of kinetic effects on the resonance behavior of the Multipole Resonance Probe

    NASA Astrophysics Data System (ADS)

    Oberrath, Jens; Mussenbrock, Thomas; Brinkmann, Ralf Peter

    2012-10-01

    Active plasma resonance spectroscopy is a well known diagnostic method. Many concepts of this method are theoretically investigated and realized as a diagnostic tool. One of these tools is the multipole resonance probe (MRP) [1]. The application of such a probe in plasmas with pressures of only a few Pa raises the question whether kinetic effects have to be taken into account or not. To address this question a kinetic model is necessary. A general kinetic model for an electrostatic concept of active plasma resonance spectroscopy has already been presented by the authors [2]. This model can be used to describe the dynamical behavior of the MRP, which is interpretable as a special case of the general model. Neglecting electron-neutral collisions, this model can be solved analytically. Based on this solution we derive an approximated expression for the admittance of the system to investigate the influence of kinetic effects on the resonance behavior of the MRP. [4pt] [1] M. Lapke et al., Plasma Sources Sci. Technol. 20, 2011, 042001[0pt] [2] J. Oberrath et al., Proceedings of the 30th International Conference on Phenomena in Ionized Gases, 28th August - 2nd September, 2011

  9. SU(4) Kondo effect in coupled quantum dots in parallel: Evidence of marginal fixed point

    NASA Astrophysics Data System (ADS)

    Eto, Mikio

    2008-03-01

    We theoretically study the Kondo effect in coupled quantum dots in parallel, using the scaling and NRG methods. The double quantum dots are capacitively coupled to each other, whereas they are attached to separate leads.ootnotetextA. Huebel, J. Weis and K.von Klitzing, 17th International Conference on the Electronic Properties of Two-Dimensional Systems (EP2DS, 2007). The SU(4) Kondo effect is realized when the energy levels are matched between the quantum dots. We show that (i) the Kondo temperature TK decreases with increasing |δ|, where δ is the level separation between the dots, obeying a power law [crossover from SU(4) to SU(2) Kondo effect]. (ii) The exponent of the power law is not a universal value in general.ootnotetextM. Eto, J. Phys. Soc. Jpn.74, 95 (2005). This is an evidence of the marginal fixed point of SU(4) Kondo effect.ootnotetextL. Borda et al., Phys. Rev. Lett. 90, 026602 (2003) (iii) The conductance through one of the quantum dots may show a non-monotonic behavior as a function of temperature T although the total conductance is a universal function of T/TK.

  10. Magnetic susceptibility of nanoscale Kondo systems

    NASA Astrophysics Data System (ADS)

    Skomski, R.; Zhang, R.; Kharel, P.; Enders, A.; Liou, S.-H.; Sellmyer, D. J.

    2010-05-01

    The mesoscopic Kondo effect in metallic nanoparticles containing a magnetic impurity is investigated by model calculations. A Maxwell-Garnett approach is used to approximately determine the resistivity of doped nanoparticles in a matrix, and the magnetic susceptibility is estimated from the confinement of the conduction electrons. Conductivity measurements of nanoparticles embedded in a matrix are difficult to realize, because metallic matrices distort the Kondo cloud, whereas insulating or semiconducting matrices yield a very weak signal. By comparison, susceptibility measurements do not suffer from these shortcomings. The Kondo effect survives in nanoparticles even if the cluster size is much smaller than the Kondo screening cloud, but the effective Curie constant becomes constant below a particle-size dependent transition temperature and the temperature dependence of the susceptibility is no longer universal.

  11. Phonon-assisted tunneling and two-channel Kondo physics in molecular junctions

    SciTech Connect

    Dias Da Silva, Luis G; Dagotto, Elbio R

    2009-01-01

    The interplay between vibrational modes and Kondo physics is a fundamental aspect of transport properties of correlated molecular conductors. We present theoretical results for a single molecule in the Kondo regime connected to left and right metallic leads, creating the usual coupling to a conduction channel with left-right parity even. A center-of-mass vibrational mode introduces an additional phonon-assisted tunneling through the antisymmetric odd channel. A non-Fermi-liquid fixed point, reminiscent of the two-channel Kondo effect, appears at a critical value of the phonon-mediated coupling strength. Our numerical renormalization-group calculations for this system reveal non-Fermi-liquid behavior at low temperatures over lines of critical points. Signatures of this strongly correlated state are prominent in the thermodynamic properties and in the linear conductance.

  12. Spatiotemporal behavior and nonlinear dynamics in a phase conjugate resonator

    NASA Technical Reports Server (NTRS)

    Liu, Siuying Raymond

    1993-01-01

    The work described can be divided into two parts. The first part is an investigation of the transient behavior and stability property of a phase conjugate resonator (PCR) below threshold. The second part is an experimental and theoretical study of the PCR's spatiotemporal dynamics above threshold. The time-dependent coupled wave equations for four-wave mixing (FWM) in a photorefractive crystal, with two distinct interaction regions caused by feedback from an ordinary mirror, was used to model the transient dynamics of a PCR below threshold. The conditions for self-oscillation were determined and the solutions were used to define the PCR's transfer function and analyze its stability. Experimental results for the buildup and decay times confirmed qualitatively the predicted behavior. Experiments were carried out above threshold to study the spatiotemporal dynamics of the PCR as a function of Pragg detuning and the resonator's Fresnel number. The existence of optical vortices in the wavefront were identified by optical interferometry. It was possible to describe the transverse dynamics and the spatiotemporal instabilities by modeling the three-dimensional-coupled wave equations in photorefractive FWM using a truncated modal expansion approach.

  13. State identification and tunable Kondo effect of MnPc on Ag(001)

    NASA Astrophysics Data System (ADS)

    Kügel, Jens; Karolak, Michael; Krönlein, Andreas; Senkpiel, Jacob; Hsu, Pin-Jui; Sangiovanni, Giorgio; Bode, Matthias

    2015-06-01

    We present a detailed investigation of spectroscopic features located at the central metal ion of MnPc (where Pc represents phthalocyanine) on Ag(001) by means of scanning tunneling spectroscopy (STS) and first-principles theory. STS data taken close to the Fermi level reveal an asymmetric feature that cannot be fitted with a single Fano function representing a one-channel Kondo effect. Instead, our data indicate the existence of a second superimposed feature. Two potential physical origins, a second Kondo channel related to the dx z /y z orbitals, and a spectral feature of the dz2 orbital itself, are discussed. A systematic experimental and theoretical comparison of MnPc with CoPc and FePc indicates that the second feature observed on MnPc is caused by the dz2 orbital. This conclusion is corroborated by STM-induced dehydrogenation experiments on FePc and MnPc which in both cases result in a gradual shift towards more positive binding energies and a narrowing of the Kondo resonance. Theoretical analysis reveals that the latter is caused by the reduced hybridization between the d orbital and the substrate. Spatially resolved differential conductivity maps taken close to the respective peak positions show that the intensity of both features is highest over the central Mn ion, thereby providing further evidence against a second Kondo channel originating from the dx z /y z orbital of the central Mn ion.

  14. Ion Behavior in an Electrically Compensated Ion Cyclotron Resonance Trap

    PubMed Central

    Brustkern, Adam M.; Rempel, Don L.; Gross, Michael L.

    2010-01-01

    We recently described a new electrically compensated trap in FT ion cyclotron resonance mass spectrometry and developed a means of tuning traps of this general design. Here, we describe a continuation of that research by comparing the ion transient lifetimes and the resulting mass resolving powers and signal-to-noise (S/N) ratios that are achievable in the compensated vs. uncompensated modes of this trap. Transient lifetimes are ten times longer under the same conditions of pressure, providing improved mass resolving power and S/N ratios. The mass resolving power as a function of m/z is linear (log-log plot) and nearly equal to the theoretical maximum. Importantly, the ion cyclotron frequency as a function of ion number decreases linearly in accord with theory, unlike its behavior in the uncompensated mode. This linearity should lead to better control in mass calibration and increased mass accuracy than achievable in the uncompensated mode. PMID:21499521

  15. Bohm-Aharonov and Kondo effects on tunneling currents in a mesoscopic ring

    SciTech Connect

    Davidovich, M.A.; Anda, E.V.; Chiappe, G.

    1997-03-01

    We present an analysis of the Kondo effect on the Bohm-Aharonov oscillations of the tunneling currents in a mesoscopic ring with a quantum dot inserted in one of its arms. The system is described by an Anderson-impurity tight-binding Hamiltonian where the electron-electron interaction is restricted to the dot. The currents are obtained using nonequilibrium Green functions calculated through a cumulant diagrammatic expansion in the chain approximation. It is shown that at low temperature, even with the system out of resonance, the Kondo peak provides a channel for the electron to tunnel through the dot, giving rise to the Bohm-Aharonov oscillations of the current. At high temperature these oscillations are important only if the dot level is aligned to the Fermi level, when the resonance condition is satisfied. {copyright} {ital 1997} {ital The American Physical Society}

  16. Kondo bahavior in antiferromagnetic NpPdSn

    NASA Astrophysics Data System (ADS)

    Shrestha, K.; Prokes, K.; Griveau, J.-C.; Jardin, R.; Colineau, E.; Caciuffo, R.; Eloirdi, R.; Gofryk, K.

    Actinide-based intermetallics show a large variety of exotic physical phenomena mainly coming from 5f hybridization with both on-site and neighboring ligand states. Depending on the strength of these process unusual behaviors such as long-range magnetic order, Kondo effect, heavy-fermion ground state, valence fluctuations, and/or superconductivity have been observed. Here we report results of our extensive studies on NpPdSn. The compound crystalizes in hexagonal ZrNiAl-type of crystal structure and is studied by means of x-ray and neutron diffraction, magnetization, heat capacity, electrical resistivity, and thermoelectric power measurements, performed over a wide range of temperatures and applied magnetic fields. All the results revealed Kondo lattice behavior and antiferromagnetic ordering below 19 K. NpPdSn can be classified as a moderately enhanced heavy-fermion system, one of very few known amidst Np-based intermetallics. Work at Idaho National Laboratory was supported by the Department of Energy, Office of Basic Energy Sciences, Materials Sciences, and Engineering Division.

  17. Effect of anisotropy in the S=1 underscreened Kondo lattice

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simões, Acirete S.; Lacroix, Claudine; Iglesias, José Roberto; Coqblin, Bernard

    2014-12-01

    We study the effect of crystal field anisotropy in the underscreened S=1 Kondo lattice model. Starting from the two orbital Anderson lattice model and including a local anisotropy term, we show, through Schrieffer-Wolff transformation, that local anisotropy is equivalent to an anisotropic Kondo interaction (J∥≠J⊥). The competition and coexistence between ferromagnetism and Kondo effect in this effective model is studied within a generalized mean-field approximation. Several regimes are obtained, depending on the parameters, exhibiting or not coexistence of magnetic order and Kondo effect. Particularly, we show that a re-entrant Kondo phase at low temperature can be obtained. We are also able to describe phases where the Kondo temperature is smaller than the Curie temperature (TKKondo effect and ferromagnetism can be understood within this model.

  18. Kondo tunneling through real and artificial molecules.

    PubMed

    Kikoin, K; Avishai, Y

    2001-03-01

    When an asymmetric double dot is hybridized with itinerant electrons, its singlet ground state and lowly excited triplet state cross, leading to a competition between the Zhang-Rice mechanism of singlet-triplet splitting in a confined cluster and the Kondo effect (which accompanies the tunneling through quantum dot under a Coulomb blockade restriction). The rich physics of an underscreened S = 1 Kondo impurity in the presence of low-lying triplet-singlet excitations is exposed and estimates of the magnetic susceptibility and the electric conductance are presented, together with applications for molecule chemisorption on metallic substrates.

  19. The physics of Kondo impurities in graphene.

    PubMed

    Fritz, Lars; Vojta, Matthias

    2013-03-01

    This article summarizes our understanding of the Kondo effect in graphene, primarily from a theoretical perspective. We shall describe different ways to create magnetic moments in graphene, either by adatom deposition or via defects. For dilute moments, the theoretical description is in terms of effective Anderson or Kondo impurity models coupled to graphene's Dirac electrons. We shall discuss in detail the physics of these models, including their quantum phase transitions and the effect of carrier doping, and confront this with existing experimental data. Finally, we will point out connections to other quantum impurity problems, e.g., in unconventional superconductors, topological insulators, and quantum spin liquids.

  20. Finite temperature topological phase transitions and emergence of Dirac semi-metallic phases in a Kondo lattice

    NASA Astrophysics Data System (ADS)

    Chou, Po-Hao; Zhai, Liang-Jun; Chung, Chung-Hou; Lee, Ting-Kuo; Mou, Chung-Yu

    The energy gap in Dirac materials controls the topology and critical behaviors of the quantum phase transition associated with the critical point when the gap vanishes. However, it is often difficult to access the critical point as it requires tunablity of electronic structures. Here by exploiting the many-body screening interaction of localized spins and conduction electrons in a Kondo lattice, we demonstrate that the electronic band structures in a Kondo lattice are tunable in temperature. When spin-orbit interactions are included, we find that below the Kondo temperature, the Kondo lattice is a strong topological insulator at low temperature and undergoes a topological transition to a weak topological insulator at a higher temperature TD. At TD, Dirac points emerge and the Kondo lattice becomes a Dirac semimetal. Our results indicate that the topological phase transition though a Dirac semi-metallic phase at finite temperatures also manifests profound physics and results in critical-like behavior both in magnetic and transport properties near TD. We acknowledge support from NCTS and Ministry of Science and Technology (MoST), Taiwan.

  1. Transport across two interacting quantum dots: Bulk Kondo, Kondo box, and molecular regimes

    NASA Astrophysics Data System (ADS)

    Costa Ribeiro, Laercio; Hamad, Ignacio; Chiappe, Guillermo; Victoriano Anda, Enrique

    2015-03-01

    We analyze the transport properties of a double quantum dot device with both dots coupled to perfect conducting leads and to a finite chain of N noninteracting sites connecting both of them. The interdot chain strongly influences the transport across the system and the local density of states of the dots. We study the case of a small number of sites, so that Kondo box effects are present, varying the coupling between the dots and the chain. For odd N and small coupling between the interdot chain and the dots, a state with two coexisting Kondo regimes develops: the bulk Kondo due to the quantum dots connected to leads and the one produced by the screening of the quantum dot spins by the spin in the finite chain at the Fermi level. As the coupling to the interdot chain increases, there is a crossover to a molecular Kondo effect, due to the screening of the molecule (formed by the finite chain and the quantum dots) spin by the leads. For even N the two Kondo temperatures regime does not develop and the physics is dominated by the usual competition between Kondo and antiferromagnetism between the quantum dots. We acknowledge financial support from the Brazilian agencies FAPERJ and CNPq.

  2. Spin fluctations and heavy fermions in the Kondo lattice

    SciTech Connect

    Khaliullin, G.G.

    1994-09-01

    This paper studies the spectrum of the spin and electronic excitations of the Kondo lattice at low temperatures. To avoid unphysical states, the Mattis {open_quotes}drone{close_quotes}-fermion representation for localized spins is employed. First, the known Fermi liquid properties of a single impurity are examined. The behavior of the correlator between a localized spin and the electron spin density at large distances shows that the effective interaction between electrons on the Fermi level and low-energy localized spin fluctuations scales as {rho}{sup {minus}1}, where {rho} is the band-state density. This fact is developed into a renormalization of the band spectrum in a periodic lattice. If the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between localized spins is much smaller than the Kondo fluctuation frequency {omega}{sub k}, the temperature of the crossover to the single-parameter Fermi liquid mode is determined by {omega}{sub k}. When the RKKY interaction becomes of order {omega}{sub k}, there is a new scale {omega}{sub sf}, the energy of the (antiferromagnetic) paramagnon mode, with {omega}{sub sf}{much_lt}{omega}{sub k}. Here the coherent Fermi liquid regime is realized only below a temperature T{sub coh} of order {omega}{sub sf}, while above T{sub coh} quasiparticle damping exhibits a linear temperature dependence. Finally, the nuclear-spin relaxation rate is calculated. 42 refs.

  3. Holographic optical traps for atom-based topological Kondo devices

    NASA Astrophysics Data System (ADS)

    Buccheri, F.; Bruce, G. D.; Trombettoni, A.; Cassettari, D.; Babujian, H.; Korepin, V. E.; Sodano, P.

    2016-07-01

    The topological Kondo (TK) model has been proposed in solid-state quantum devices as a way to realize non-Fermi liquid behaviors in a controllable setting. Another motivation behind the TK model proposal is the demand to demonstrate the quantum dynamical properties of Majorana fermions, which are at the heart of their potential use in topological quantum computation. Here we consider a junction of crossed Tonks-Girardeau gases arranged in a star-geometry (forming a Y-junction), and we perform a theoretical analysis of this system showing that it provides a physical realization of the TK model in the realm of cold atom systems. Using computer-generated holography, we experimentally implement a Y-junction suitable for atom trapping, with controllable and independent parameters. The junction and the transverse size of the atom waveguides are of the order of 5 μm, leading to favorable estimates for the Kondo temperature and for the coupling across the junction. Since our results show that all the required theoretical and experimental ingredients are available, this provides the demonstration of an ultracold atom device that may in principle exhibit the TK effect.

  4. Holographic optical traps for atom-based topological Kondo devices

    NASA Astrophysics Data System (ADS)

    Buccheri, F.; Bruce, G. D.; Trombettoni, A.; Cassettari, D.; Babujian, H.; Korepin, V. E.; Sodano, P.

    2016-07-01

    The topological Kondo (TK) model has been proposed in solid-state quantum devices as a way to realize non-Fermi liquid behaviors in a controllable setting. Another motivation behind the TK model proposal is the demand to demonstrate the quantum dynamical properties of Majorana fermions, which are at the heart of their potential use in topological quantum computation. Here we consider a junction of crossed Tonks–Girardeau gases arranged in a star-geometry (forming a Y-junction), and we perform a theoretical analysis of this system showing that it provides a physical realization of the TK model in the realm of cold atom systems. Using computer-generated holography, we experimentally implement a Y-junction suitable for atom trapping, with controllable and independent parameters. The junction and the transverse size of the atom waveguides are of the order of 5 μm, leading to favorable estimates for the Kondo temperature and for the coupling across the junction. Since our results show that all the required theoretical and experimental ingredients are available, this provides the demonstration of an ultracold atom device that may in principle exhibit the TK effect.

  5. Non-Kondo zero-bias anomaly in disordered quantum wires

    SciTech Connect

    Wen, Chong-Shian; Hsiao, J. H.; Chen, Jeng-Chung

    2014-02-14

    We investigated the behavior of the zero-bias anomaly in quantum wires that were embedded with impurities. The linear conductance G can exhibit cusp features that evolve with the positions of the impurities, and these features can be continuously changed using a combination of spit-gate and top-gate voltages. ZBA is observed regardless of the presence of impurity. Kondo model is inadequate for describing the behaviors of both G and ZBA. Despite the presence of impurity scattering, various ZBA behaviors that resemble those reported in clean quantum wires can be observed. Our results suggest that ZBA is an intrinsic phenomenon in a quantum wire, and its temperature and magnetic field dependence does not pertain to the Kondo correlations in quantum dot.

  6. Unexpected observation of spatially separated Kondo scattering and ferromagnetism in Ta alloyed anatase TiO2 thin films

    PubMed Central

    Sarkar, T. P.; Gopinadhan, K.; Motapothula, M.; Saha, S.; Huang, Z.; Dhar, S.; Patra, A.; Lu, W. M.; Telesio, F.; Pallecchi, I.; Ariando; Marré, D.; Venkatesan, T.

    2015-01-01

    We report the observation of spatially separated Kondo scattering and ferromagnetism in anatase Ta0.06Ti0.94O2 thin films as a function of thickness (10–200 nm). The Kondo behavior observed in thicker films is suppressed on decreasing thickness and vanishes below ~25 nm. In 200 nm film, transport data could be fitted to a renormalization group theory for Kondo scattering though the carrier density in this system is lower by two orders of magnitude, the magnetic entity concentration is larger by a similar magnitude and there is strong electronic correlation compared to a conventional system such as Cu with magnetic impurities. However, ferromagnetism is observed at all thicknesses with magnetic moment per unit thickness decreasing beyond 10 nm film thickness. The simultaneous presence of Kondo and ferromagnetism is explained by the spatial variation of defects from the interface to surface which results in a dominantly ferromagnetic region closer to substrate-film interface while the Kondo scattering is dominant near the surface and decreasing towards the interface. This material system enables us to study the effect of neighboring presence of two competing magnetic phenomena and the possibility for tuning them. PMID:26265554

  7. On the zero-bias anomaly and Kondo physics in quantum point contacts near pinch-off.

    PubMed

    Xiang, S; Xiao, S; Fuji, K; Shibuya, K; Endo, T; Yumoto, N; Morimoto, T; Aoki, N; Bird, J P; Ochiai, Y

    2014-03-26

    We investigate the linear and non-linear conductance of quantum point contacts (QPCs), in the region near pinch-off where Kondo physics has previously been connected to the appearance of the 0.7 feature. In studies of seven different QPCs, fabricated in the same high-mobility GaAs/AlGaAs heterojunction, the linear conductance is widely found to show the presence of the 0.7 feature. The differential conductance, on the other hand, does not generally exhibit the zero-bias anomaly (ZBA) that has been proposed to indicate the Kondo effect. Indeed, even in the small subset of QPCs found to exhibit such an anomaly, the linear conductance does not always follow the universal temperature-dependent scaling behavior expected for the Kondo effect. Taken collectively, our observations demonstrate that, unlike the 0.7 feature, the ZBA is not a generic feature of low-temperature QPC conduction. We furthermore conclude that the mere observation of the ZBA alone is insufficient evidence for concluding that Kondo physics is active. While we do not rule out the possibility that the Kondo effect may occur in QPCs, our results appear to indicate that its observation requires a very strict set of conditions to be satisfied. This should be contrasted with the case of the 0.7 feature, which has been apparent since the earliest experimental investigations of QPC transport.

  8. Resonance behavior of single ultrathin slot antennas on finite dielectric substrates in terahertz regime

    NASA Astrophysics Data System (ADS)

    Park, H. R.; Koo, S. M.; Suwal, O. K.; Park, Y. M.; Kyoung, J. S.; Seo, M. A.; Choi, S. S.; Park, N. K.; Kim, D. S.; Ahn, K. J.

    2010-05-01

    We investigate resonance behaviors of optically thin metallic slot antennas on finite substrates in terahertz frequency regime. By carefully analyzing theoretical and experimental results, we observe that slot antennas fabricated in a gold film with a thickness below the skin depth of gold show blueshifted resonance frequencies for the increasing slot width, while the opposite resonance behaviors appear when the slot antennas are perforated in perfectly electric conductor. In addition, we find that for slot antenna sustained by a finite substrate its thickness and the slot width are additional crucial factors determining the resonance frequency of slot antennas.

  9. A molecular approach to the Kondo problem in Carbon based systems

    NASA Astrophysics Data System (ADS)

    Soriano, Maria; Jacob, David; Palacios, Juan Jose

    2014-03-01

    There has been a great effort in recent years to understand the emerging Kondo-like resonances in different magnetic molecules such as MnPc. Theoretical approaches based on atomic models have proven to be very useful for the study of this phenomenon when the magnetic moment is essentially localized on a magnetic atom. Nevertheless the Kondo effect can arise in pure carbon-based systems as has been demonstrated experimentally in fullerenes and carbon nanotubes. In this communication we present a multiorbital Anderson model where the orbitals are not atomic but molecular orbitals. This model is fully obtained from Density Functional Theory calculation in combination with Green's functions methodologies. Standard impurity solver techniques are used to solve the model which is applied to fullerenes and other nanographene structures.

  10. A fully first-principles approach to the Molecular Kondo problem

    NASA Astrophysics Data System (ADS)

    Soriano, Maria; Jacob, David; Palacios, Juan José; Atomelix Team

    2015-03-01

    There has been a great effort in recent years to understand the emerging Kondo-like resonances in different magnetic molecules such as MnPc. Theoretical approaches based on atomic models have proven to be very useful for the study of this phenomenon when the magnetic moment is essentially localized on a magnetic atom. Nevertheless the Kondo effect can arise in pure carbon-based systems as has been demonstrated experimentally in fullerenes and carbon nanotubes. In this communication we present a multiorbital Anderson model where the orbitals are not atomic but molecular orbitals. This model is fully obtained from Density Functional Theory calculation in combination with Green's functions methodologies. Standard impurity solver techniques are used to solve the model which is applied to fullerenes and other nanographene structures.

  11. Interplay between the Kondo effect and the Ruderman-Kittel-Kasuya-Yosida interaction.

    PubMed

    Prüser, Henning; Dargel, Piet E; Bouhassoune, Mohammed; Ulbrich, Rainer G; Pruschke, Thomas; Lounis, Samir; Wenderoth, Martin

    2014-11-11

    The interplay between the Ruderman-Kittel-Kasuya-Yosida interaction and the Kondo effect is expected to provide the driving force for the emergence of many phenomena in strongly correlated electron materials. Two magnetic impurities in a metal are the smallest possible system containing all these ingredients and define a bottom-up approach towards a long-term understanding of concentrated/dense systems. Here we report on the experimental and theoretical investigation of iron dimers buried below a Cu(100) surface by means of low-temperature scanning tunnelling spectroscopy combined with density functional theory and numerical renormalization group calculations. The Kondo effect, in particular the width of the Abrikosov-Suhl resonance, is strongly altered or even suppressed due to magnetic coupling between the impurities. It oscillates as a function of dimer separation revealing that it is related to indirect exchange interactions mediated by the conduction electrons.

  12. Maximized orbital and spin Kondo effects in a single-electron transistor

    NASA Astrophysics Data System (ADS)

    Le Hur, Karyn; Simon, Pascal; Borda, László

    2004-01-01

    We investigate the charge fluctuations of a single-electron box (metallic grain) coupled to a lead via a smaller quantum dot in the Kondo regime. The most interesting aspect of this problem resides in the interplay between spin Kondo physics stemming from the screening of the spin of the small dot and orbital Kondo physics emerging when charging states of the grain with (charge) Q=0 and Q=e are almost degenerate. Combining Wilson’s numerical renormalization-group method with perturbative scaling approaches we push forward our previous work [K. Le Hur and P. Simon, Phys. Rev. B 67, 201308R (2003)]. We emphasize that, for symmetric and slightly asymmetric barriers, the strong entanglement of charge and spin flip events in this setup inevitably results in a nontrivial stable SU(4) Kondo fixed point near the degeneracy points of the grain. By analogy with a small dot sandwiched between two leads, the ground state is Fermi-liquid-like, which considerably smears out the Coulomb staircase behavior and prevents the Matveev logarithmic singularity from arising. Most notably, the associated Kondo temperature TSU(4)K might be raised compared to that in conductance experiments through a small quantum dot (˜1 K), which makes the observation of our predictions a priori accessible. We discuss the robustness of the SU(4) correlated state against the inclusion of an external magnetic field, a deviation from the degeneracy points, particle-hole symmetry in the small dot, and asymmetric tunnel junctions and comment on the different crossovers.

  13. Dynamical symmetries in Kondo tunneling through complex quantum dots.

    PubMed

    Kuzmenko, T; Kikoin, K; Avishai, Y

    2002-10-01

    Kondo tunneling reveals hidden SO(n) dynamical symmetries of evenly occupied quantum dots. As is exemplified for an experimentally realizable triple quantum dot in parallel geometry, the possible values n=3,4,5,7 can be easily tuned by gate voltages. Following construction of the corresponding o(n) algebras, scaling equations are derived and Kondo temperatures are calculated. The symmetry group for a magnetic field induced anisotropic Kondo tunneling is SU(2) or SO(4).

  14. Linear and nonlinear behavior of crystalline optical whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy A.; Matsko, Andrey B.; Ilchenko, Vladimir S.; Maleki, Lute

    2004-01-01

    We demonstrate strong nonlinear behavior of high-Q whispering gallery mode (WGM) resonators made out of various crystals adn devices based on the resonators. The maximum WGM optical Q-fact or achieved at room temperature exceeds 2X10 to the tenth power.

  15. Kondo effect and STM spectroscopy of Dirac electrons in graphene

    NASA Astrophysics Data System (ADS)

    Sengupta, Krishnendu

    2011-03-01

    We show that graphene, whose low-energy quasiparticles display Dirac like behavior, may exhibit a two-channel Kondo effect in the presence of magnetic impurities. We present a large N analysis for a generic spin S local moment coupled to Dirac electrons in graphene and demonstrate that the corresponding Kondo temperature can be tuned by an experimentally controllable applied gate voltage. We also study the STM spectra of these Dirac electrons in the presence of such impurities and demonstrate that such spectra depend qualitatively on the position of the impurity atom in the graphene matrix. More specifically, for impurity atoms atop the hexagon center, the zero-bias tunneling conductance, as measured by a STM, shows a peak; for those atop a graphene site, it shows a dip. We provide a qualitative theoretical explanation of this phenomenon and show that this unconventional behavior is a consequence of conservation/breaking of pseudospin symmetry of the Dirac quasiparticles by the impurity. We also predict that tuning the Fermi energy to zero by a gate voltage would not lead to qualitative change in the shape of the conductance spectra when the impurity is atop the hexagon center. A similar tuning of the Fermi energy for the impurity atop a site, however, would lead to a change in the tunneling conductance from a dip to a peak via an antiresonance. We discuss some recent experiments on a doped graphene sample that seem to have qualitative agreement with our theory and suggest further experiments to test our predictions. DST, India.

  16. Kondo Effect at a Quantum Critical Point

    NASA Astrophysics Data System (ADS)

    Ramazashvili, Revaz; Coleman, Piers

    1998-03-01

    The Kondo effect in a metal on the verge of a zero-temperature magnetic instability provides a fascinating example of interference between local and long-range correlations. (A. I. Larkin and V. I. Mel'nikov, Sov. Phys. JETP 34, 656 (1972)) (P. Coleman and A. M. Tsvelik, cond-mat/9707003) (A. Sengupta, cond-mat/9707316) We discuss possible consequences of this interference, including the breakdown of the Fermi liquid state.

  17. Kondo effects in triangular triple quantum dots

    NASA Astrophysics Data System (ADS)

    Oguri, Akira; Numata, Takahide; Nisikawa, Yunori; Hewson, A. C.

    2009-03-01

    We study the conductance through a triangular triple quantum dot, which is connected to two noninteracting leads, using the numerical renormalization group (NRG). It is found that the system shows a variety of Kondo effects depending on the filling of the triangle. The SU(4) Kondo effect occurs at half-filling, and a sharp conductance dip due to a phase lapse appears in the gate-voltage dependence. Furthermore, when four electrons occupy the three sites on average, a local S=1 moment, which is caused by the Nagaoka mechanism, is induced along the triangle. The temperature dependence of the entropy and spin susceptibility of the triangle shows that this moment is screened by the conduction electrons via two separate stages at different temperatures. The two-terminal and four-terminal conductances show a clear difference at the gate voltages, where the SU(4) or the S=1 Kondo effects occur[1]. We will also discuss effects of deformations of the triangular configuration, caused by the inhomogeneity in the inter-dot couplings and in the gate voltages. [4pt] [1] T.Numata, Y.Nisikawa, A.Oguri, and A.C.Hewson: arXiv:0808.3496.

  18. Stochastic resonance in psychophysics and in animal behavior.

    PubMed

    Ward, Lawrence M; Neiman, Alexander; Moss, Frank

    2002-08-01

    A recent analysis of the energy detector model in sensory psychophysics concluded that stochastic resonance does not occur in a measure of signal detectability ( d'), but can occur in a percent-correct measure of performance as an epiphenomenon of nonoptimal criterion placement [Tougaard (2000) Biol Cybern 83: 471-480]. When generalized to signal detection in sensory systems in general, this conclusion is a serious challenge to the idea that stochastic resonance could play a significant role in sensory processing in humans and other animals. It also seems to be inconsistent with recent demonstrations of stochastic resonance in sensory systems of both nonhuman animals and humans using measures of system performance such as signal-to-noise ratio of power spectral densities and percent-correct detections in a two-interval forced-choice paradigm, both closely related to d'. In this paper we address this apparent dilemma by discussing several models of how stochastic resonance can arise in signal detection systems, including especially those that implement a "soft threshold" at the input transform stage. One example involves redefining d' for energy increments in terms of parameters of the spike-count distribution of FitzHugh-Nagumo neurons. Another involves a Poisson spike generator that receives an exponentially transformed noisy periodic signal. In this case it can be shown that the signal-to-noise ratio of the power spectral density at the signal frequency, which exhibits stochastic resonance, is proportional to d'. Finally, a variant of d' is shown to exhibit stochastic resonance when calculated directly from the distributions of power spectral densities at the signal frequency resulting from transformation of noise alone and a noisy signal by a sufficiently steep nonlinear response function. All of these examples, and others from the literature, imply that stochastic resonance is more than an epiphenomenon, although significant limitations to the extent to which

  19. Anisotropy induced Kondo splitting in a mechanically stretched molecular junction: A first-principles based study.

    PubMed

    Wang, Xiaoli; Hou, Dong; Zheng, Xiao; Yan, YiJing

    2016-01-21

    The magnetic anisotropy and Kondo phenomena in a mechanically stretched magnetic molecular junction are investigated by combining the density functional theory (DFT) and hierarchical equations of motion (HEOM) approach. The system is comprised of a magnetic complex Co(tpy-SH)2 sandwiched between adjacent gold electrodes, which is mechanically stretched in experiments done by Parks et al. [Science 328, 1370 (2010)]. The electronic structure and mechanical property of the stretched system are investigated via the DFT calculations. The HEOM approach is then employed to characterize the Kondo resonance features, based on the Anderson impurity model parameterized from the DFT results. It is confirmed that the ground state prefers the S = 1 local spin state. The structural properties, the magnetic anisotropy, and corresponding Kondo peak splitting in the axial stretching process are systematically evaluated. The results reveal that the strong electron correlations and the local magnetic properties of the molecule magnet are very sensitive to structural distortion. This work demonstrates that the combined DFT+HEOM approach could be useful in understanding and designing mechanically controlled molecular junctions.

  20. Photoemission and the electronic properties of heavy fermions -- limitations of the Kondo model

    SciTech Connect

    Joyce, J.J.; Arko, A.J.; Andrews, A.B.

    1993-09-01

    The electronic properties of Yb-based heavy fermions have been investigated by means of high resolution synchrotron radiation photoemission and compared with predictions of the Kondo model. The Yb heavy fermion photoemission spectra show massive disagreement with the Kondo model predictions (as calculated within the Gunnarsson-Schonhammer computational method). Moreover, the Yb heavy fermion photoemission spectra give very strong indications of core-like characteristics and compare favorable to purely divalent Yb metal and core-like Lu 4f levels. The heavy fermions YbCu{sub 2}Si{sub 2}, YbAgCu{sub 4} and YbAl{sub 3} were measured and shown to have lineshapes much broader and deeper in binding energy than predicted by the Kondo model. The lineshape of the bulk component of the 4f emission for these three heavy fermion materials was compared with that from Yb metal and the Lu 4f levels in LuAl{sub 3}, the heavy fermion materials show no substantive spectroscopic differences from simple 4f levels observed in Yb metal and LuAl{sub 3}. Also, the variation with temperature of the 4f fineshape was measured for Yb metal and clearly demonstrates that phonon broadening plays a major role in 4f level lineshape analysis and must be accounted for before considerations of correlated electron resonance effects are presumed to be at work.

  1. Robust topological surface state in Kondo insulator SmB{sub 6} thin films

    SciTech Connect

    Yong, Jie Jiang, Yeping; Zhang, Xiaohang; Greene, Richard L.; Usanmaz, Demet; Curtarolo, Stefano; Li, Linze; Pan, Xiaoqing; Shin, Jongmoon; Takeuchi, Ichiro

    2014-12-01

    Fabrication of smooth thin films of topological insulators with true insulating bulk are extremely important for utilizing their novel properties in quantum and spintronic devices. Here, we report the growth of crystalline thin films of SmB{sub 6}, a topological Kondo insulator with true insulating bulk, by co-sputtering both SmB{sub 6} and B targets. X-ray diffraction, Raman spectroscopy, and transmission electron microscopy indicate films that are polycrystalline with a (001) preferred orientation. When cooling down, resistivity ρ shows an increase around 50 K and saturation below 10 K, consistent with the opening of the hybridization gap and surface dominated transport, respectively. The ratio ρ{sub 2K}/ρ{sub 300K} is only about two, much smaller than that of bulk, which indicates a much larger surface-to-bulk ratio. Point contact spectroscopy using a superconductor tip on SmB{sub 6} films shows both a Kondo Fano resonance and Andeev reflection, indicating an insulating Kondo lattice with metallic surface states.

  2. Interpreting the behavior of a quarter-wave transmission line resonator in a magnetized plasma

    SciTech Connect

    Gogna, G. S. Turner, M. M.; Karkari, S. K.

    2014-12-15

    The quarter wave resonator immersed in a strongly magnetized plasma displays two possible resonances occurring either below or above its resonance frequency in vacuum, f{sub o}. This fact was demonstrated in our recent articles [G. S. Gogna and S. K. Karkari, Appl. Phys. Lett. 96, 151503 (2010); S. K. Karkari, G. S. Gogna, D. Boilson, M. M. Turner, and A. Simonin, Contrib. Plasma Phys. 50(9), 903 (2010)], where the experiments were carried out over a limited range of magnetic fields at a constant electron density, n{sub e}. In this paper, we present the observation of dual resonances occurring over the frequency scan and find that n{sub e} calculated by considering the lower resonance frequency is 25%–30% smaller than that calculated using the upper resonance frequency with respect to f{sub o}. At a given magnetic field strength, the resonances tend to shift away from f{sub o} as the background density is increased. The lower resonance tends to saturate when its value approaches electron cyclotron frequency, f{sub ce}. Interpretation of these resonance conditions are revisited by examining the behavior of the resonance frequency response as a function of n{sub e}. A qualitative discussion is presented which highlights the practical application of the hairpin resonator for interpreting n{sub e} in a strongly magnetized plasma.

  3. Interpreting the behavior of a quarter-wave transmission line resonator in a magnetized plasma

    NASA Astrophysics Data System (ADS)

    Gogna, G. S.; Karkari, S. K.; Turner, M. M.

    2014-12-01

    The quarter wave resonator immersed in a strongly magnetized plasma displays two possible resonances occurring either below or above its resonance frequency in vacuum, fo. This fact was demonstrated in our recent articles [G. S. Gogna and S. K. Karkari, Appl. Phys. Lett. 96, 151503 (2010); S. K. Karkari, G. S. Gogna, D. Boilson, M. M. Turner, and A. Simonin, Contrib. Plasma Phys. 50(9), 903 (2010)], where the experiments were carried out over a limited range of magnetic fields at a constant electron density, ne. In this paper, we present the observation of dual resonances occurring over the frequency scan and find that ne calculated by considering the lower resonance frequency is 25%-30% smaller than that calculated using the upper resonance frequency with respect to fo. At a given magnetic field strength, the resonances tend to shift away from fo as the background density is increased. The lower resonance tends to saturate when its value approaches electron cyclotron frequency, fce. Interpretation of these resonance conditions are revisited by examining the behavior of the resonance frequency response as a function of ne. A qualitative discussion is presented which highlights the practical application of the hairpin resonator for interpreting ne in a strongly magnetized plasma.

  4. Mass-Imbalanced Superconductivity in Effective Two-Channel Kondo Lattice

    NASA Astrophysics Data System (ADS)

    Kusunose, Hiroaki

    2016-11-01

    We propose that mass-imbalanced superconductivity is realized in an effective two-channel Kondo lattice, and its characteristic property appears in electromagnetic responses such as the Meissner effect. Starting from an effective two-channel Kondo lattice model as a low-energy effective theory, and approximating it with two mean-field order parameter components in a self-consistent fashion, it is shown that the balance of the two components is sensitively reflected in the magnitude of the Meissner kernel, while thermodynamic properties are little affected by the balance. This remarkable behavior is understood by the localized character of one partner in the Cooper pair, namely, the effect of the mass imbalance. We briefly mention the relevance to the huge enhancement of the upper critical field under pressure observed in Pr 1-2-20 systems.

  5. Magnetic frustration in itinerant systems: the Kondo polaron problem

    NASA Astrophysics Data System (ADS)

    Isaev, Leonid; Batista, Cristian; Vekhter, Ilya

    2013-03-01

    We study the interplay between magnetic frustration and Kondo screening in Kondo lattices by analyzing the J1-J2 antiferromagnetic chain coupled to a conduction band. The system is tuned to the Majumdar-Ghosh point J2 =J1 / 2 which stabilizes a dimer valence-bond solid at weak Kondo coupling JK. We use an effective low-energy theory to demonstrate that sufficiently large JK results in a proliferation of ``Kondo polarons'', i.e. Kondo-screened domain-wall excitations of the dimer state, and collapse of the dimer order via a 2nd order quantum phase transition. At the quantum critical point, JK =JKc , these polarons become gapless, and we argue that the transition itself belongs to a 2D Ising universality class. For JK >JKc increasing concentration of the polarons leads to a continuous growth of the electron Fermi momentum until all spins are absorbed by the Fermi sea.

  6. Kondo interactions from band reconstruction in YbInCu4

    SciTech Connect

    Jarrige, I.; Kotani, A.; Yamaoka, H.; Tsujii, N.; Ishii, K.; Upton, M.; Casa, D.; Kim, J.; Gog, T.; Hancock, J. N.

    2015-03-27

    We combine resonant inelastic X-ray scattering (RIXS) and model calculations in the Kondo lattice compound YbInCu₄, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T≃42 K. In this study, the bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasi-gap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system.

  7. Kondo Effect in a Single Electron Transistor

    NASA Astrophysics Data System (ADS)

    Goldhaber-Gordon, David

    1998-03-01

    When a field-effect transistor is made very small, and electrons in the channel are separated from those in the leads by tunnel junctions, the transistor turns on and off every time an extra electron is added to the channel. The droplet of electrons confined in the channel of such a single-electron transistor (SET) interacts with electrons in the leads. This is in close analogy to an impurity atom interacting with the delocalized electrons in a metal, the traditional system for studying the Kondo effect.(Y. Meir, N.S. Wingreen, and P.A. Lee. PRL) 70, 2601 (1993) I will discuss measurements on a new generation of SETs that display all the aspects of the Kondo effect:(D. Goldhaber-Gordon, Hadas Shtrikman, D. Mahalu, D. Abusch-Magder, U. Meirav, and M.A. Kastner. To be published in Nature). a spin singlet forms between a localized electron in the channel and delocalized electrons in the leads, causing an enhancement of the zero-bias conductance, when the number of electrons on the artificial atom is odd but not when it is even. The system can be studied out of equilibrium by applying a voltage between the two leads, an impossible procedure in bulk Kondo systems. The spin singlet is altered by applying such a voltage or a magnetic field or by increasing the temperature, all in ways that agree with predictions. In addition, the tunability of an SET allows study of the system over a range of parameters not easily accessible to previous calculations or experiments.

  8. Two-channel Kondo effect and phonon-assisted transport in single-molecular junctions

    NASA Astrophysics Data System (ADS)

    Dias da Silva, Luis; Dagotto, Elbio

    2009-03-01

    The interplay between vibrational modes and Kondo physics is a fundamental aspect of transport properties of correlated molecular conductors. In this theoretical work, we study such interplay in a system consisting of a single molecule in a metallic break junction tuned (by gate voltages) to be in an ``odd-N'' coulomb blockade valley (Kondo-prone). The connection to left and right metallic leads creates the usual coupling to a conduction channel with left-right symmetry (the ``even"-parity channel). A center-of-mass vibrational mode introduces an additional, phonon-assisted tunneling through the asymmetric (``odd''-parity channel). Our numerical renormalization-group calculations reveal that the phonon-mediated coupling to the odd channel leads to the appearance of a two-channel Kondo (2chK) effect, characterized by a non-Fermi-liquid (NFL) fixed point. The ground-state has NFL properties for a critical value of the phonon-mediated coupling strength and critical lines are present for wide range of parameters, including the regime away from particle-hole symmetry. Signatures of this 2chK non-Fermi-liquid behavior are prominent in the thermodynamic properties as well as in the linear conductance.

  9. Interplay between Kondo screening and local singlets in SU (N) -symmetric cold atoms

    NASA Astrophysics Data System (ADS)

    Isaev, Leonid; Rey, Ana Maria

    2015-03-01

    We study collective phenomena in strongly interacting fermionic alkaline-earth atoms (AEAs) loaded in an optical lattice. Owing to the strong decoupling between electronic orbital and nuclear-spin degrees of freedom, AEAs prepared in the two lowest electronic states are predicted to obey an accurate SU (N > 2 I + 1) symmetry in their two-body collisions (I is the nuclear spin). The SU (N) symmetric models offer a great opportunity to generate exotic many-body behavior emerging from the increased degeneracy and strict conservation laws. We focus on a parameter regime that realizes an SU (N > 2) (Coqblin-Schrieffer) generalization of the usual Kondo lattice model, and show that for band fillings above one atom per site, the system exhibits a peculiar interplay between Kondo screening and formation of singlets between localized atoms. In the limit of large Kondo coupling, we derive an effective Hamiltonian and determine its phase diagram. Our results can be tested in experiments with ultracold 173 Yb or 87 Sr atoms and are relevant for the physics of heavy-fermion materials with magnetic frustration. Supported by AFOSR, MURI-AFOSR and NSF.

  10. Natural orbitals renormalization group approach to the two-impurity Kondo critical point

    NASA Astrophysics Data System (ADS)

    He, Rong-Qiang; Dai, Jianhui; Lu, Zhong-Yi

    2015-04-01

    The problem of two magnetic impurities in a normal metal exposes the two opposite tendencies in the formation of a singlet ground state, driven respectively by the single-ion Kondo effect with conduction electrons to screen impurity spins or the Ruderman-Kittel-Kasuya-Yosida interaction between the two impurities to directly form impurity spin singlet. However, whether the competition between these two tendencies can lead to a quantum critical point has been debated over more than two decades. Here, we study this problem by applying the newly proposed natural orbitals renormalization group method to a lattice version of the two-impurity Kondo model with a direct exchange K between the two impurity spins. The method allows for unbiased access to the ground state wave functions and low-lying excitations for sufficiently large system sizes. We demonstrate the existence of a quantum critical point, characterized by the power-law divergence of impurity staggered susceptibility with critical exponent γ =0.60 (1 ) , on the antiferromagnetic side of K when the interimpurity distance R is even lattice spacing, while a crossover behavior is recovered when R is odd lattice spacing. These results have ultimately resolved the long-standing discrepancy between the numerical renormalization group and quantum Monte Carlo studies, confirming a link of this two-impurity Kondo critical point to a hidden particle-hole symmetry predicted by the local Fermi liquid theory.

  11. Analysis of the Kane-Mele-Kondo lattice at finite temperatures

    NASA Astrophysics Data System (ADS)

    Yoshida, Tsuneya; Peters, Robert; Kawakami, Norio

    Recently, correlation effects on topological insulators are extensively studied because the interplay of topological properties and electron correlations is expected to induce exotic phenomena. A promising candidate for a topological insulator in heavy-fermion systems is ∖mathrmSmB6 where the Kondo effects play an essential role. In this article, we study the Kane-Mele-Kondo lattice at finite temperatures. By using the dynamical mean-field theory, we obtain a temperature vs. interaction phase diagram (a Doniach phase diagram). Furthermore, we have observed an intriguing crossover behavior induced by the interplay of electron correlations and topologically nontrivial properties. In the bulk system, the spin-Hall conductivity which is proportional to the spin Chern number is zero at low temperatures while the conductivity rapidly increases with increasing temperature. Correspondingly, gapless modes are restored by temperature effects at the edge sites, which are destroyed by the Kondo effect at low temperature. This work is partly supported by KAKENHI (No. 25400366, and 15H05855). The numerical calculations were performed at the ISSP in the University of Tokyo and on the SR16000 at YITP in Kyoto University.

  12. Calculation of the quasi-energies and resonances behavior of the hydrogen Lyman-alpha problem

    NASA Technical Reports Server (NTRS)

    Ruyten, Wilhelmus M.

    1992-01-01

    Recently, Bakshi and Kalman presented numerical results for the quasi-energies of the n = 2 multiplet in the hydrogen Lyman-alpha transition for a plasma in which both strong static and oscillating electric fields are present. Recent work on related magnetic and optical resonance problems provides a simplified mathematical treatment, as well as greater insight into the complex resonance behavior of this interaction.

  13. Numerical analysis of the spatial range of the Kondo effect

    SciTech Connect

    Busser, C. A.; Martins, G. B.; Ribeiro, L. Costa; Vernek, E.; Anda, E. V.; Dagotto, Elbio R

    2010-01-01

    The spatial length of the Kondo screening is still a controversial issue related to Kondo physics. While renormalization-group and Bethe-Ansatz solutions have provided detailed information about the thermodynamics of magnetic impurities, they are insufficient to study the effect on the surrounding electrons, i.e., the spatial range of the correlations created by the Kondo effect between the localized magnetic moment and the conduction electrons. The objective of this work is to present a quantitative way of measuring the extension of these correlations by studying their effect directly on the local density of states (LDOS) at arbitrary distances from the impurity. The numerical techniques used, the embedded cluster approximation, the finite-U slave bosons, and numerical renormalization group, calculate the Green s functions in real space. With this information, one can calculate how the local density of states away from the impurity is modified by its presence, below and above the Kondo temperature, and then estimate the range of the disturbances in the noninteracting Fermi sea due to the Kondo effect, and how it changes with the Kondo temperature TK. The results obtained agree with results obtained through spin-spin correlations, showing that the LDOS captures the phenomenology of the Kondo cloud as well.

  14. Intracavity Beam Behavior in Hybrid Resonator Planar-Waveguide CO(2) Lasers.

    PubMed

    Wasilewski, B; Baker, H J; Hall, D R

    2000-11-20

    We describe a combined computer simulation and experimental investigation of the intracavity spatial beam profile characteristics of a planar-waveguide rf-excited CO(2) laser that incorporates a hybrid waveguide confocal unstable negative-branch resonator. The study includes results for the intracavity lateral beam intensity profile and output power of the laser as a function of resonator mirror misalignment. In addition, the behavior of the unstable resonator, observed experimentally and predicted by the simulation, in generating localized high intensity hot-spots when it is subjected to relatively large misalignment angles is reported. PMID:18354625

  15. Kondo Effect in CeXc (Xc = S, Se, Te) Studied by Electrical Resistivity Measurements under High Pressure

    NASA Astrophysics Data System (ADS)

    Hayashi, Yuya; Takai, Shun; Matsumura, Takeshi; Tanida, Hiroshi; Sera, Masafumi; Matsubayashi, Kazuyuki; Uwatoko, Yoshiya; Ochiai, Akira

    2016-03-01

    We have measured the electrical resistivity of cerium monochalcogenides, CeS, CeSe, and CeTe, under high pressures of up to 8 GPa. The pressure dependences of the antiferromagnetic ordering temperature TN, crystal field splitting, and the ln T anomaly of the Kondo effect have been studied to cover the entire region from the magnetic ordering regime at low pressure to the Fermi liquid regime at high pressure. TN initially increases with increasing pressure, and starts to decrease at high pressure as expected from Doniach’s diagram. Simultaneously, the ln T behavior in the resistivity is enhanced, indicating the enhancement of the Kondo effect by pressure. It is also characteristic of CeXc that the crystal field splitting rapidly decreases at a common rate of -12.2 K/GPa. This leads to the increase in the degeneracy of the f state and the further enhancement of the Kondo effect. It is shown that the pressure-dependent degeneracy of the f state is a key factor for understanding the pressure dependence of TN, the Kondo effect, magnetoresistance, and the peak structure in the temperature dependence of resistivity.

  16. Collective behavior of globally coupled Langevin equations with colored noise in the presence of stochastic resonance

    NASA Astrophysics Data System (ADS)

    Yang, Bo; Zhang, Xiao; Zhang, Lu; Luo, Mao-Kang

    2016-08-01

    The long-time collective behavior of globally coupled Langevin equations in a dichotomous fluctuating potential driven by a periodic source is investigated. By describing the collective behavior using the moments of the mean field and single-particle displacements, we study stochastic resonance and synchronization using the exact steady-state solutions and related stability criteria. Based on the simulation results and the criterion of the stationary regime, the notable differences between the stationary and nonstationary regimes are demonstrated. For the stationary regime, stochastic resonance with synchronization is discussed, and for the nonstationary regime, the volatility clustering phenomenon is observed.

  17. Microwave memristive behavior in split-ring resonator metamaterials

    NASA Astrophysics Data System (ADS)

    Wu, H. Y.; Shi, S. K.; Wang, C. H.; Jiang, X. J.; Yu, G.; Qin, G. Q.; Fu, H.; Zhou, J.

    2016-07-01

    Photonic memristors, which behave as memristors operating with electromagnetic fields, present an effective means to achieve all-optical networking, and can promote the development of optical communications and computer technology. In this paper, we report a microwave memristive phenomenon at room temperature in metamaterials consisting of negative temperature coefficient thermistor ceramic disk and split-ring resonator (SRR). Hysteretic transmission-incident field power loops, the area of which varies with the scan rate of power, (similar to the fingerprint of memristors) were observed in the metamaterials. These effects are attributed to the increasing conductivity of the ceramic disk with increasing temperature generated by the interaction between electromagnetic waves and metamaterials. This work offers new opportunities for the development of photonic memristors.

  18. Spin dynamics and Kondo physics in optical tweezers

    NASA Astrophysics Data System (ADS)

    Lin, Yiheng; Lester, Brian J.; Brown, Mark O.; Kaufman, Adam M.; Long, Junling; Ball, Randall J.; Isaev, Leonid; Wall, Michael L.; Rey, Ana Maria; Regal, Cindy A.

    2016-05-01

    We propose to use optical tweezers as a toolset for direct observation of the interplay between quantum statistics, kinetic energy and interactions, and thus implement minimum instances of the Kondo lattice model in systems with few bosonic rubidium atoms. By taking advantage of strong local exchange interactions, our ability to tune the spin-dependent potential shifts between the two wells and complete control over spin and motional degrees of freedom, we design an adiabatic tunneling scheme that efficiently creates a spin-singlet state in one well starting from two initially separated atoms (one atom per tweezer) in opposite spin state. For three atoms in a double-well, two localized in the lowest vibrational mode of each tweezer and one atom in an excited delocalized state, we plan to use similar techniques and observe resonant transfer of two-atom singlet-triplet states between the wells in the regime when the exchange coupling exceeds the mobile atom hopping. Moreover, we argue that such three-atom double-tweezers could potentially be used for quantum computation by encoding logical qubits in collective spin and motional degrees of freedom. Current address: Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.

  19. Fano-Andreev effect in Quantum Dots in Kondo regime

    NASA Astrophysics Data System (ADS)

    Orellana, Pedro; Calle, Ana Maria; Pacheco, Monica; Apel, Victor

    In the present work, we investigate the transport through a T-shaped double quantum dot system coupled to two normal leads and to a superconducting lead. We study the role of the superconducting lead in the quantum interferometric features of the double quantum dot and by means of a slave boson mean field approximation at low temperature regime. We inquire into the influence of intradot interactions in the electronic properties of the system as well. Our results show that Fano resonances due to Andreev bound states are exhibited in the transmission from normal to normal lead as a consequence of quantum interference and proximity effect. This Fano effect produced by Andreev bound states in a side quantum dot was called Fano-Andreev effect, which remains valid even if the electron-electron interaction are taken into account, that is, the Fano-Andreev effect is robust against e-e interactions even in Kondo regime. We acknowledge the financial support from FONDECYT program Grants No. 3140053 and 11400571.

  20. Coexistence of Kondo effect and ferromagnetism in the Underscreened Kondo Lattice model

    NASA Astrophysics Data System (ADS)

    Thomas, C.; Simões, A. S. R.; Iglesias, J. R.; Lacroix, C.; Perkins, N. B.; Coqblin, B.

    2011-12-01

    In this work we use a Schrieffer-Wolff transformation in a two-fold degenerate periodic Anderson lattice to describe the coexistence of Kondo effect and ferromagnetism in some uranium and neptunium compounds. We show that the inclusion of a bandwidth for the f electrons can account for a weak delocalization of 5f electrons. Using a mean field approximation, we show that a maximum of TC versus JK can be found when the bandwidth is proportional to JK.

  1. Observation of orbital two-channel Kondo effect in a ferromagnetic L10-MnGa film

    NASA Astrophysics Data System (ADS)

    Zhu, Lijun; Woltersdorf, Georg; Zhao, Jianhua

    2016-09-01

    The experimental existence and stability of the fixed point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics have been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system resonant scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and a square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, respectively. Our results not only evidence the robust existence of orbital 2CK effect even in the presence of strong magnetic fields and long-range ferromagnetic ordering, but also extend the scope of 2CK host materials from nonmagnetic nanoscale point contacts to diffusive conductors of disordered alloys.

  2. Observation of orbital two-channel Kondo effect in a ferromagnetic L10-MnGa film

    PubMed Central

    Zhu, Lijun; Woltersdorf, Georg; Zhao, Jianhua

    2016-01-01

    The experimental existence and stability of the fixed point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics have been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system resonant scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and a square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, respectively. Our results not only evidence the robust existence of orbital 2CK effect even in the presence of strong magnetic fields and long-range ferromagnetic ordering, but also extend the scope of 2CK host materials from nonmagnetic nanoscale point contacts to diffusive conductors of disordered alloys. PMID:27686323

  3. Universal spatial correlations in the anisotropic Kondo screening cloud: Analytical insights and numerically exact results from a coherent state expansion

    NASA Astrophysics Data System (ADS)

    Florens, Serge; Snyman, Izak

    2015-11-01

    We analyze the spatial correlation structure of the spin density of an electron gas in the vicinity of an antiferromagnetically coupled Kondo impurity. Our analysis extends to the regime of spin-anisotropic couplings, where there are no quantitative results for spatial correlations in the literature. We use an original and numerically exact method, based on a systematic coherent-state expansion of the ground state of the underlying spin-boson Hamiltonian. It has not yet been applied to the computation of observables that are specific to the fermionic Kondo model. We also present an important technical improvement to the method that obviates the need to discretize modes of the Fermi sea, and allows one to tackle the problem in the thermodynamic limit. As a result, one can obtain excellent spatial resolution over arbitrary length scales, for a relatively low computational cost, a feature that gives the method an advantage over popular techniques such as the numerical and density-matrix renormalization groups. We find that the anisotropic Kondo model shows rich universal scaling behavior in the spatial structure of the entanglement cloud. First, SU(2) spin-symmetry is dynamically restored in a finite domain in the parameter space in the vicinity of the isotropic line, as expected from poor man's scaling. More surprisingly, we are able to obtain in closed analytical form a set of different, yet universal, scaling curves for strong exchange asymmetry, which are parametrized by the longitudinal exchange coupling. Deep inside the cloud, i.e., for distances smaller than the Kondo length, the correlation between the electron spin density and the impurity spin oscillates between ferromagnetic and antiferromagnetic values at the scale of the Fermi wavelength, an effect that is drastically enhanced at strongly anisotropic couplings. Our results also provide further numerical checks and alternative analytical approximations for the Kondo overlaps that were recently computed by

  4. Resonant-state expansions and the long-time behavior of quantum decay

    SciTech Connect

    Garcia-Calderon, Gaston; Maldonado, Irene; Villavicencio, Jorge

    2007-07-15

    It is shown that a representation of the decaying wave function as a resonant sum plus a nonexponential integral term may be written as a purely discrete resonant sum by evaluating at long times the integral term by the steepest descents method, and then expanding the resulting expression in terms of resonant states. This leads to a representation that is valid along the exponential and the inverse power in time regimes. A model calculation using the {delta} potential allows us to make a comparison of the expansion with numerical integrations in terms of continuum wave functions and, in the long time regime, with an exact analytic expression of the integral term obtained using the steepest descents method. The results demonstrate that resonant states give a correct description of the long-time behavior of decay.

  5. Nonlinear resonant behavior of a dispersive readout circuit for a superconducting flux qubit

    NASA Astrophysics Data System (ADS)

    Lee, Janice C.; Oliver, William D.; Berggren, Karl K.; Orlando, T. P.

    2007-04-01

    A nonlinear resonant circuit comprising a SQUID magnetometer and a shunting capacitor is studied as a readout scheme for a persistent-current qubit. The flux state of the qubit is detected as a change in the Josephson inductance of the SQUID magnetometer, which in turn mediates a shift in the resonant frequency of the readout circuit. The nonlinearity and resulting hysteresis in the resonant behavior are characterized as a function of the power of both the input drive and the associated resonance-peak response. Numerical simulations based on a nonlinear circuit model shows that the observed nonlinearity is dominated by the effect due to an ac flux rather than current bias through the Josephson inductor.

  6. Ray-optical calculation of eigenmode behavior of unstable laser resonators with rounded edges.

    PubMed

    Santana, C

    1981-08-15

    The eigenmode resonance equation, previously developed by the ray-optical method of analysis for unstable symmetric bare resonators with strip and spherical mirrors, is employed here to establish the basic properties of resonators with rounded mirror edges. The numerical results obtained in this manner are far more comprehensive than those presented earlier from a waveguide model approach to the resonator problem. As in this earlier study, edge rounding is found to improve mode separation and to shift the onset of low-loss mode detachment to lower Fresnel numbers. It is also found that a simple closed form expression predicts accurately the low-loss mode behavior after it has detached from the remaining mode spectrum. PMID:20333052

  7. Modulating resonance behaviors by noise recycling in bistable systems with time delay

    SciTech Connect

    Sun, Zhongkui Xu, Wei; Yang, Xiaoli; Xiao, Yuzhu

    2014-06-01

    In this paper, the impact of noise recycling on resonance behaviors is studied theoretically and numerically in a prototypical bistable system with delayed feedback. According to the interior cooperating and interacting activity of noise recycling, a theory has been proposed by reducing the non-Markovian problem into a two-state model, wherein both the master equation and the transition rates depend on not only the current state but also the earlier two states due to the recycling lag and the feedback delay. By virtue of this theory, the formulae of the power spectrum density and the linear response function have been found analytically. And the theoretical results are well verified by numerical simulations. It has been demonstrated that both the recycling lag and the feedback delay play a crucial role in the resonance behaviors. In addition, the results also suggest an alternative scheme to modulate or control the coherence or stochastic resonance in bistable systems with time delay.

  8. Multichannel Kondo impurity dynamics in a Majorana device.

    PubMed

    Altland, A; Béri, B; Egger, R; Tsvelik, A M

    2014-08-15

    We study the multichannel Kondo impurity dynamics realized in a mesoscopic superconducting island connected to metallic leads. The effective "impurity spin" is nonlocally realized by Majorana bound states and strongly coupled to lead electrons by non-Fermi liquid correlations. We explore the spin dynamics and its observable ramifications near the low-temperature fixed point. The topological protection of the system raises the perspective to observe multichannel Kondo impurity dynamics in experimentally realistic environments.

  9. Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2

    PubMed Central

    Aynajian, Pegor; da Silva Neto, Eduardo H.; Parker, Colin V.; Huang, Yingkai; Pasupathy, Abhay; Mydosh, John; Yazdani, Ali

    2010-01-01

    Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu2Si2. We find that, as the temperature is lowered, partial screening of the f electrons’ spins gives rise to a spatially modulated Kondo–Fano resonance that is maximal between the surface U atoms. At T = 17.5 K, URu2Si2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states. PMID:20498090

  10. MEAN MOTION RESONANCES IN EXOPLANET SYSTEMS: AN INVESTIGATION INTO NODDING BEHAVIOR

    SciTech Connect

    Ketchum, Jacob A.; Adams, Fred C.; Bloch, Anthony M.

    2013-01-10

    Motivated by the large number of extrasolar planetary systems that are near mean motion resonances, this paper explores a related type of dynamical behavior known as 'nodding'. Here, the resonance angle of a planetary system executes libration (oscillatory motion) for several cycles, circulates for one or more cycles, and then enters once again into libration. This type of complicated dynamics can affect our interpretation of observed planetary systems that are in or near mean motion resonance. This work shows that planetary systems in (near) mean motion resonance can exhibit nodding behavior, and outlines the portion of parameter space where it occurs. This problem is addressed using both full numerical integrations of the planetary systems and via model equations obtained through expansions of the disturbing function. In the latter approach, we identify the relevant terms that allow for nodding. The two approaches are in agreement, and show that nodding often occurs when a small body is in an external mean motion resonance with a larger planet. As a result, the nodding phenomenon can be important for interpreting observations of transit timing variations, where the existence of smaller bodies is inferred through their effects on larger, observed transiting planets. For example, in actively nodding planetary systems, both the amplitude and frequency of the transit timing variations depend on the observational time window.

  11. Mean Motion Resonances in Exoplanet Systems: An Investigation into Nodding Behavior

    NASA Astrophysics Data System (ADS)

    Ketchum, Jacob A.; Adams, Fred C.; Bloch, Anthony M.

    2013-01-01

    Motivated by the large number of extrasolar planetary systems that are near mean motion resonances, this paper explores a related type of dynamical behavior known as "nodding." Here, the resonance angle of a planetary system executes libration (oscillatory motion) for several cycles, circulates for one or more cycles, and then enters once again into libration. This type of complicated dynamics can affect our interpretation of observed planetary systems that are in or near mean motion resonance. This work shows that planetary systems in (near) mean motion resonance can exhibit nodding behavior, and outlines the portion of parameter space where it occurs. This problem is addressed using both full numerical integrations of the planetary systems and via model equations obtained through expansions of the disturbing function. In the latter approach, we identify the relevant terms that allow for nodding. The two approaches are in agreement, and show that nodding often occurs when a small body is in an external mean motion resonance with a larger planet. As a result, the nodding phenomenon can be important for interpreting observations of transit timing variations, where the existence of smaller bodies is inferred through their effects on larger, observed transiting planets. For example, in actively nodding planetary systems, both the amplitude and frequency of the transit timing variations depend on the observational time window.

  12. {ital Ab Initio} Calculation of Crystalline Electric Fields and Kondo Temperatures in Ce Compounds

    SciTech Connect

    Han, J.; Alouani, M.; Cox, D.; Han, J.; Cox, D.; Alouani, M.

    1997-02-01

    We have calculated the band-f hybridizations for Ce{sub x}La{sub 1-x}M{sub 3} compounds (x=1 and x{r_arrow}0; M=Pb,In,Sn,Pd) within the local density approximation and fed this into a noncrossing approximation for the Anderson impurity model applied to both dilute and concentrated limits. Our calculations produce crystalline electric field splittings and Kondo temperatures with trends in good agreement with experiment and demonstrate the need for detailed electronic structure information on hybridization to describe the diverse behaviors of these Ce compounds. {copyright} {ital 1997} {ital The American Physical Society}

  13. Extraordinary Hall effect in Kondo-type systems: Contributions from anomalous velocity

    NASA Astrophysics Data System (ADS)

    Levy, P. M.

    1988-10-01

    Kondo systems exhibit a relatively large extraordinary Hall effect which is due to asymmetric resonant scattering of conduction electrons. Theories based on the skew scattering mechanism account for data at high temperatures T>TK (the Kondo temperature) but are unable to explain the very-low-temperature variation of the Hall constant observed in heavy-fermion compounds. Aside from the ordinary Hall effect, caused by the Lorentz force and skew scattering (which makes the scattering probability antisymmetric with respect to interchange of scattering vectors), there exists an additional contribution to the Hall effect known as the anomalous-velocity contribution. This contribution is due to a change in the expression for the current operator in the presence of spin-orbit forces. We derive an expression for the anomalous velocity in terms of the T matrices describing conduction-electron scattering; it is not limited to weak spin-orbit scattering as were previous results. We use the Anderson model of local moments in metals to write this scattering in terms of the mixing interaction between local and conduction electrons, and the local state's Green's function. The transverse Hall current due to anomalous velocity is determined and evaluated in two limits. At high temperature, we use the weak-coupling form of the local state's Green's function; at T=0 K a phase-shift analysis is used, and we rely on the Friedel-Langreth sum rule to give us the phase shift at the Fermi surface. At high temperatures we find that the contribution from anomalous velocity to the Hall constant is quite small compared to that from skew scattering. On the contrary, at low temperatures the anomalous velocity makes the dominant contribution to the Hall constant in Kondo systems.

  14. Local Kondo screening and spatial coherence in YbRh2Si2

    NASA Astrophysics Data System (ADS)

    Wirth, Steffen

    2012-02-01

    Heavy fermion metals are often characterized by a variety of relevant energy scales and competing interactions which may result in such fascinating phenomena as quantum criticality and unconventional superconductivity. Therefore, these materials have advanced to suitable model systems by means of which electronic interactions can be studied in detail. This will be discussed for the interplay of localized and itinerant electronic states in Kondo lattice systems in which heavy charge carriers are generated. We investigate the generic Kondo lattice system YbRh2Si2, one of the heaviest heavy fermion metals, by utilizing atomically resolved Scanning Tunneling Spectroscopy (STS) [1]. An analysis of the topography allows for a determination of the terminating surface as well as a comparison to results from chemical analysis. Importantly, the crystal field excitations are unambiguously reflected by our STS measurements, clearly relating STS to bulk properties. The hybridization of conduction and 4f electrons results in a gap-like feature in the tunneling conductance. In addition, a strongly temperature dependent peak in the tunneling conductance is attributed to a resonance resulting from the Kondo lattice. The experimental data are discussed in relation to results obtained within the non-crossing approximation (NCA) and renormalized band structure calculation. In a brief outlook we discuss further investigations by STS, e.g. with respect to the quantum critical phenomena observed in YbRh2Si2 [2], to substitutions-induced changes of the relevant energy scales [3], or on heavy fermion superconductors. [4pt] [1] S. Ernst et al., Nature 474 (2011) 362.[0pt] [2] S. Friedemann et al., Proc. Natl. Acad. Sci. USA 107 (2010) 14547.[0pt] [3] S. Friedemann et al., Nature Phys. 5 (2009) 465.

  15. Visualizing heavy fermions emerging in a quantum critical Kondo lattice

    NASA Astrophysics Data System (ADS)

    Aynajian, Pegor

    2013-03-01

    In solids containing elements with f orbitals, the interaction between f-electron spins and those of itinerant electrons leads to the development of low-energy fermionic excitations with a heavy effective mass. These excitations are fundamental to the appearance of unconventional superconductivity and non-Fermi-liquid behavior observed in actinide- and lanthanide-based compounds. We use spectroscopic mapping with the scanning tunneling microscope to detect the emergence of heavy excitations with lowering of temperature in a prototypical family of cerium-based heavy-fermion compounds. We demonstrate the sensitivity of the tunneling process to the composite nature of these heavy quasiparticles, which arises from quantum entanglement of itinerant conduction and f electrons. Scattering and interference of the composite quasiparticles is used to resolve their energy-momentum structure and to extract their mass enhancement, which develops with decreasing temperature. The lifetime of the emergent heavy quasiparticles reveals signatures of enhanced scattering and their spectral lineshape shows evidence of energy-temperature scaling. These findings demonstrate that proximity to a quantum critical point results in critical damping of the emergent heavy excitation of our Kondo lattice system. This work is funded by a DOE-BES grant. Partial support for instrumentation is provided by NSF-DMR, Keck Foundation, and NSF-MRSEC. PA also acknowledges support of a fellowship through the PCCM funded by NSF MERSEC.

  16. Resonance induced spin-selective transport behavior in carbon nanoribbon/nanotube/nanoribbon heterojunctions

    NASA Astrophysics Data System (ADS)

    Zhang, Xiang-Hua; Wang, Ling-Ling; Li, Xiao-Fei; Chen, Tong; Li, Quan

    2015-09-01

    Carbon nanotubes (CNTs) and graphene nanoribbons (GNRs) are attractive in spintronics. Here, we propose GNR/CNT/GNR heterojunctions constructed by attaching zigzag-GNRs at the side-wall of CNT for spintronic devices. The thermal stability and electronic transport properties were explored using ab initio molecular dynamics simulations and nonequilibrium Green's function methods, respectively. Results demonstrate that the sp3-hybridized contacts formed at the interface assure a good thermal stability of the system and make the CNT to be regarded as resonator. Only the electron of one spin-orientation and resonant energy is allowed to transport, resulting in the remarkable spin-selective transport behavior at the ferromagnetic state.

  17. Majorana modes and Kondo effect in a quantum dot attached to a topological superconducting wire (Presentation Recording)

    NASA Astrophysics Data System (ADS)

    Vernek, Edson; Ruiz-Tijerina, David; da Silva, Luis D.; Egues, José Carlos

    2015-09-01

    Quantum dot attached to topological wires has become an interesting setup to study Majorana bound state in condensed matter[1]. One of the major advantage of using a quantum dot for this purpose is that it provides a suitable manner to study the interplay between Majorana bound states and the Kondo effect. Recently we have shown that a non-interacting quantum dot side-connected to a 1D topological superconductor and to metallic normal leads can sustain a Majorana mode even when the dot is empty. This is due to the Majorana bound state of the wire leaking into the quantum dot. Now we investigate the system for the case in which the quantum dot is interacting[3]. We explore the signatures of a Majorana zero-mode leaking into the quantum dot, using a recursive Green's function approach. We then study the Kondo regime using numerical renormalization group calculations. In this regime, we show that a "0.5" contribution to the conductance appears in system due to the presence of the Majorana mode, and that it persists for a wide range of the dot parameters. In the particle-hole symmetric point, in which the Kondo effect is more robust, the total conductance reaches 3e^2/2h, clearly indicating the coexistence of a Majorana mode and the Kondo resonance in the dot. However, the Kondo effect is suppressed by a gate voltage that detunes the dot from its particle-hole symmetric point as well as by a Zeeman field. The Majorana mode, on the other hand, is almost insensitive to both of them. We show that the zero-bias conductance as a function of the magnetic field follows a well-known universal curve. This can be observed experimentally, and we propose that this universality followed by a persistent conductance of 0.5,e^2/h are evidence for the presence of Majorana-Kondo physics. This work is supported by the Brazilians agencies FAPESP, CNPq and FAPEMIG. [1] A. Y. Kitaev, Ann.Phys. {bf 303}, 2 (2003). [2] E. Vernek, P.H. Penteado, A. C. Seridonio, J. C. Egues, Phys. Rev. B {bf

  18. Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6

    SciTech Connect

    Fuhrman, W. T.; Leiner, Jonathan C.; Nikolić, P.; Granroth, Garrett E.; Stone, Matthew B.; Lumsden, Mark D.; DeBeer-Schmitt, Lisa M.; Alekseev, Pavel A.; Mignot, Jean-Michel; Koohpayeh, S. M.; Cottingham, P.; Phelan, William Adam; Schoop, L.; McQueen, T. M.; Broholm, C.

    2015-01-21

    In this paper, using inelastic neutron scattering, we map a 14 meV coherent resonant mode in the topological Kondo insulator SmB6 and describe its relation to the low energy insulating band structure. The resonant intensity is confined to the X and R high symmetry points, repeating outside the first Brillouin zone and dispersing less than 2 meV, with a 5d-like magnetic form factor. We present a slave-boson treatment of the Anderson Hamiltonian with a third neighbor dominated hybridized band structure. This approach produces a spin exciton below the charge gap with features that are consistent with the observed neutron scattering. Finally, we find that maxima in the wave vector dependence of the inelastic neutron scattering indicate band inversion.

  19. Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6

    DOE PAGES

    Fuhrman, W. T.; Leiner, Jonathan C.; Nikolić, P.; Granroth, Garrett E.; Stone, Matthew B.; Lumsden, Mark D.; DeBeer-Schmitt, Lisa M.; Alekseev, Pavel A.; Mignot, Jean-Michel; Koohpayeh, S. M.; et al

    2015-01-21

    In this paper, using inelastic neutron scattering, we map a 14 meV coherent resonant mode in the topological Kondo insulator SmB6 and describe its relation to the low energy insulating band structure. The resonant intensity is confined to the X and R high symmetry points, repeating outside the first Brillouin zone and dispersing less than 2 meV, with a 5d-like magnetic form factor. We present a slave-boson treatment of the Anderson Hamiltonian with a third neighbor dominated hybridized band structure. This approach produces a spin exciton below the charge gap with features that are consistent with the observed neutron scattering.more » Finally, we find that maxima in the wave vector dependence of the inelastic neutron scattering indicate band inversion.« less

  20. Dielectric relaxation, resonance and scaling behaviors in Sr3Co2Fe24O41 hexaferrite.

    PubMed

    Tang, Rujun; Jiang, Chen; Qian, Wenhu; Jian, Jie; Zhang, Xin; Wang, Haiyan; Yang, Hao

    2015-08-28

    The dielectric properties of Z-type hexaferrite Sr3Co2Fe24O41 (SCFO) have been investigated as a function of temperature from 153 to 503 K between 1 and 2 GHz. The dielectric responses of SCFO are found to be frequency dependent and thermally activated. The relaxation-type dielectric behavior is observed to be dominating in the low frequency region and resonance-type dielectric behavior is found to be dominating above 10(8) Hz. This frequency dependence of dielectric behavior is explained by the damped harmonic oscillator model with temperature dependent coefficients. The imaginary part of impedance (Z″) and modulus (M″) spectra show that there is a distribution of relaxation times. The scaling behaviors of Z″ and M″ spectra further suggest that the distribution of relaxation times is temperature independent at low frequencies. The dielectric loss spectra at different temperatures have not shown a scaling behavior above 10(8) Hz. A comparison between the Z″ and the M″ spectra indicates that the short-range charges motion dominates at low temperatures and the long-range charges motion dominates at high temperatures. The above results indicate that the dielectric dispersion mechanism in SCFO is temperature independent at low frequencies and temperature dependent at high frequencies due to the domination of resonance behavior.

  1. Vibration-mediated Kondo transport in molecular junctions: conductance evolution during mechanical stretching

    PubMed Central

    Rakhmilevitch, David

    2015-01-01

    Summary The vibration-mediated Kondo effect attracted considerable theoretical interest during the last decade. However, due to lack of extensive experimental demonstrations, the fine details of the phenomenon were not addressed. Here, we analyze the evolution of vibration-mediated Kondo effect in molecular junctions during mechanical stretching. The described analysis reveals the different contributions of Kondo and inelastic transport. PMID:26734532

  2. Enhancement of Kondo effect through Rashba spin-orbit interactions

    NASA Astrophysics Data System (ADS)

    Sandler, Nancy; Zarea, Mehdi; Ulloa, Sergio

    2011-03-01

    The role of Rashba spin-orbit (RSO) interactions on the Kondo regime has been a topic of debate since resistivity measurements on Pt doped Cu:Mn compounds were interpreted as evidence for suppression of the Kondo effect by SO scattering. Subsequent theoretical and experimental activity has yielded conflicting results. Thus, the question: what is the role of SO interactions in the Kondo regime? remains open. To provide a definite answer we obtain an exact solution of an Anderson magnetic impurity model in a two-dimensional metallic host with RSO interactions. We show that the Hamiltonian reduces to an effective two-band Anderson model coupled to a S=1/2 impurity. An appropriate Schrieffer-Wolff transformation produces an effective 2-channel Kondo model plus a Dzyaloshiinski-Moriya (DM) interaction term. The exact solution reveals that the impurity couples to the bath with ferro- and antiferromagnetic couplings. DM interactions, that vanish at half-filling and at the Hubbard U-infinity limits, introduce an exponential increase in the value of the Kondo temperature. Supported by NSF-PIRE and MWN/CIAM.

  3. Magnetic impurities in Cu nanocontacts: Kondo effect and conductance from first principles

    NASA Astrophysics Data System (ADS)

    Jacob, David; Haule, Kristjan; Kotliar, Gabriel

    2009-03-01

    We present ab initio calculations of the electronic structure and coherent transport properties of Cu nanocontacts hosting a single magnetic impurity (Fe,Co or Ni) in the contact region. The strong electron correlations of the impurity 3d-electrons are fully taken into account by combining density functional calculations with a dynamical treatment of the impurity 3d-shell in the so called one-crossing approximation. We find that for all three impurities the strong electron correlations give rise to Kondo resonances at the Fermi level which in turn lead to Fano lineshapes in the coherent transport characteristics of the nanocontact. The exact shape of the Kondo and Fano lineshapes, however, depends strongly on the impurity type and the geometry of the contact. This is in agreement with recent experiments measuring the conductance of magnetic impurities on noble metal surfaces [1-4]. [1] P. Wahl et al., Phys. Rev. Lett. 93, 176603 (2004). [2] N. N'eel et al., Phys. Rev. Lett. 98, 016801 (2007). [3] L. Vitali et al., Phys. Rev. Lett. 101, 216802 (2008). [4] N. N'eel et al., arXiv:0810.0236 (2008).

  4. Spin-glass freezing above the ordering temperature for the Kondo ferromagnet CeNi{sub 0.4}Cu{sub 0.6}

    SciTech Connect

    Gomez Sal, J.C.; Garcia Soldevilla, J.; Blanco, J.A.; Espeso, J.I.; Rodriguez Fernandez, J.; Luis, F.; Bartolome, F.; Bartolome, J.

    1997-11-01

    The low-temperature magnetic and transport properties of the orthorhombic CeNi{sub 0.4}Cu{sub 0.6} compound have been determined from the analysis of specific heat, ac magnetic susceptibility, electrical resistivity, elastic and inelastic neutron scattering. These measurements present intriguing experimental results that could not be explained within the usual phenomenology of Ce-based compounds. C{sub p} and {chi}{sub ac} present anomalies around 1 K corresponding to ferromagnetic order as confirmed by neutron diffraction. The magnetic structure is collinear with very reduced moments, 0.6{mu}{sub B}/Ce lying in the b direction. Additionally, a clear Kondo behavior is observed with a Kondo temperature T{sub K}=1.9K estimated from quasielastic neutron scattering. Above the ordering temperature, further anomalies are observed in C{sub p} and {chi}{sub ac} that could not be explained as originating from crystal electric field or Kondo effects. From the frequency and field dependence of the {chi}{sub ac}, above T{sub c}, a spin-glass state with a freezing temperature T{sub f}=2K is proposed for this compound. This unusual magnetic behavior is discussed in terms of mixed (positive and negative) Ruderman-Kittel-Kasuya-Yosida interactions, randomness (structural disorder), large hybridization (Kondo effect), and strong magnetocrystalline anisotropy (crystal electric field effects). {copyright} {ital 1997} {ital The American Physical Society}

  5. Kondo phase transitions of magnetic impurities in carbon nanotubes

    NASA Astrophysics Data System (ADS)

    Fang, Tie-Feng; Sun, Qing-feng

    2013-02-01

    We propose carbon nanotubes (CNTs) with magnetic impurities as a versatile platform to achieve exciting Kondo physics, where the CNT bath is gapped by the spin-orbit interaction and renormalized by interference effects. While the strong-coupling phase is inaccessible for the special case of half-filled impurities in neutral armchair CNTs, the system in general can undergo quantum phase transitions to the Kondo ground state. The resultant position-specific phase diagrams are investigated upon variation of the CNT radius, chirality, and carrier doping, revealing several striking features, e.g., the existence of a maximal radius for nonarmchair CNTs to realize phase transitions, and an interference-induced suppression of the Kondo screening. We show that by tuning the Fermi energy via electrostatic gating, the quantum critical region can be experimentally accessed.

  6. Quadrupolar Kondo effect in uranium heavy-electron materials?

    NASA Technical Reports Server (NTRS)

    Cox, D. L.

    1987-01-01

    The possibility of an electric quadrupole Kondo effect for a non-Kramers doublet on a uranium (U) ion is a cubic metallic host is demonstrated by model calculations showing a Kondo upturn in the resistivity, universal quenching of the quadrupolar moment, and a heavy-electron anomaly in the electronic specific heat. With inclusion of excited crystal-field levels, some of the unusual magnetic-response data in the heavy-electron superconductor UBe13 may be understood. Structural phase transitions at unprecedented low temperatures may occur in U-based heavy-electron materials.

  7. The entanglement structure of the Kondo singlet in energy space

    NASA Astrophysics Data System (ADS)

    Yang, Chun; Feiguin, Adrian

    We unveil the entanglement structure of the Kondo singlet in energy space by studying the contribution of each individual free electron eigenstate. This is a problem of two spins coupled to a bath, where the bath is formed by the remaining conduction electrons. Being a mixed state, we resort to the ''concurrence'' as a good measure of entanglement. Using the density matrix renormalization group and analytical variational calculations with the Yoshida wave-function, and slave bosons, we find a distinct transition between weak and strong coupling regimes characterized by very different entanglement distributions. We discuss implications to the theory of the Kondo cloud.

  8. Inelastic transport through Aharonov-Bohm interferometer in Kondo regime

    SciTech Connect

    Yoshii, Ryosuke; Eto, Mikio; Sakano, Rui; Affleck, Ian

    2013-12-04

    We formulate elastic and inelastic parts of linear conductance through an Aharonov-Bohm (AB) ring with an embedded quantum dot in the Kondo regime. The inelastic part G{sub inel} is proportional to T{sup 2} when the temperature T is much smaller than the Kondo temperature T{sub K}, whereas it is negligibly small compared with elastic part G{sub el} when T ≫ T{sub K}. G{sub inel} weakly depends on the magnetic flux penetrating the AB ring, which disturbs the precise detection of G{sub el}/(G{sub el}+G{sub inel}) by the visibility of AB oscillation.

  9. Tunneling spectroscopy of a single quantum dot coupled to a superconductor: From Kondo ridge to Andreev bound states

    NASA Astrophysics Data System (ADS)

    Pillet, J.-D.; Joyez, P.; Žitko, Rok; Goffman, M. F.

    2013-07-01

    We performed tunneling spectroscopy of a carbon nanotube quantum dot (QD) coupled to a metallic reservoir either in the normal or in the superconducting state. We explore how the Kondo resonance, observed when the QD's occupancy is odd and the reservoir is normal, evolves towards Andreev bound states (ABS) in the superconducting state. Within this regime, the ABS spectrum observed is consistent with a quantum phase transition from a singlet to a degenerate magnetic doublet ground state, in quantitative agreement with a single-level Anderson model with superconducting leads.

  10. The spin glass-antiferromagnetism competition in Kondo-lattice systems in the presence of a transverse applied magnetic field

    NASA Astrophysics Data System (ADS)

    Magalhaes, S. G.; Zimmer, F. M.; Coqblin, B.

    2006-05-01

    A theory is proposed to describe the competition among antiferromagnetism (AF), spin glass (SG) and Kondo effect. The model describes two Kondo sublattices with an intrasite Kondo interaction strength JK and a random Gaussian interlattice interaction in the presence of a transverse field Γ. The Γ field is introduced as a quantum mechanism to produce spin flipping and the random coupling has average -2J0/N and variance 32J2/N. The path integral formalism with Grassmann fields is used to study this fermionic problem, in which the disorder is treated within the framework of the replica trick. The free energy and the order parameters are obtained using the static ansatz. In this many parameters problem, we choose J0/J≈(JK/J)2 and Γ/J≈(JK/J)2 to allow a better comparison with the experimental findings. The obtained phase diagram has not only the same sequence as the experimental one for Ce2Au1-xCoxSi3, but mainly, it also shows a qualitative agreement concerning the behavior of the freezing temperature and the Neel temperature which decreases until a quantum critical point (QCP).

  11. Constructive influence of the induced electron pairing on the Kondo state

    PubMed Central

    Domański, T.; Weymann, I.; Barańska, M.; Górski, G.

    2016-01-01

    Superconducting order and magnetic impurities are usually detrimental to each other. We show, however, that in nanoscopic objects the induced electron pairing can have constructive influence on the Kondo effect originating from the effective screening interactions. Such situation is possible at low temperatures in the quantum dots placed between the conducting and superconducting reservoirs, where the proximity induced electron pairing cooperates with the correlations amplifying the spin-exchange potential. The emerging Abrikosov-Suhl resonance, which is observable in the Andreev conductance, can be significantly enhanced by increasing the coupling to superconducting lead. We explain this intriguing tendency within the Anderson impurity model using: the generalized Schrieffer-Wolff canonical transformation, the second order perturbative treatment of the Coulomb repulsion, and the nonperturbative numerical renormalization group calculations. We also provide hints for experimental observability of this phenomenon. PMID:27009681

  12. Is the black phase of SmS a topological Kondo insulator?

    NASA Astrophysics Data System (ADS)

    Bauer, Eric; Ghimire, N. J.; Ronning, F.; Batista, C.; Byler, D.; Thompson, J. D.; Rahmanisisan, A.; Fisk, Z.

    2015-03-01

    SmS is a prototypical Kondo insulator where electronic correlations drive a system insulating that would otherwise be metallic. Whether or not such a system is also a topological insulator that hosts a protected metallic surface state, depends on the parity of the wavefunction of the occupied states. However, unlike weakly correlated materials, it is unclear whether state-of-the-art electronic structure calculations accurately predict the parity of the occupied wavefunctions of correlated insulators. Nevertheless, Dzero and collaborators suggest that Kondo insulators such as SmB6 can be topological. Like SmB6, Cubic SmS is a non-magnetic semiconductor with an insulating behavior at ambient pressure and low temperatures driven by hybridization with the Sm f-electrons. At 6 kbar, SmS undergoes a phase transition into a valance fluctuating phase accompanied by a visible color change from black to gold. It then undergoes a second phase transition at about 20 kbar to an antiferromagnetic order at low temperatures. We will discuss whether electronic structure calculations indicate a topological state of SmS at P =0. We will also discuss whether or not the magnetic, thermal and transport properties of the black phase of SmS are consistent with the existence of a topological protected surface state.

  13. Critical-field theory of the Kondo lattice model in two dimensions

    SciTech Connect

    Kim, Ki-Seok

    2005-05-15

    In the context of the U(1) slave-boson theory we derive a critical-field theory near the quantum-critical point of the Kondo lattice model in two spatial dimensions. First, we argue that strong gauge fluctuations in the U(1) slave-boson theory give rise to confinement between spinons and holons, thus causing 'neutralized' spinons in association with the slave-boson U(1) gauge field. Second, we show that critical fluctuations of Kondo singlets near the quantum-critical point result in a new U(1) gauge field. This emergent gauge field has nothing to do with the slave-boson U(1) gauge field. Third, we find that the slave-boson U(1) gauge field can be exactly integrated out in the low-energy limit. As a result we find a critical-field theory in terms of renormalized conduction electrons and neutralized spinons interacting via the new emergent U(1) gauge field. Based on this critical-field theory we obtain the temperature dependence of the specific heat and the imaginary part of the self-energy of the renormalized electrons. These quantities display non-Fermi-liquid behavior near the quantum-critical point.

  14. Spin Alignment and Resonance Behavior in the Magnesium -24 + MAGNESIUM-24 System.

    NASA Astrophysics Data System (ADS)

    Wuosmaa, Alan Harrison

    1988-12-01

    We have studied heavy-ion resonance behavior in the ^{24}Mg + ^{24}Mg system using particle- gamma and particle-gamma -gamma angular correlation techniques. These methods have allowed us to determine the single and correlated magnetic-substate populations for single and mutual inelastic scattering to the 2 ^+(1.37 MeV) state in ^{24 }Mg in the region of two strong resonances seen at E_{c.m} = 45.70 and 46.65 MeV^1. Our measurements were performed using the Holifield Heavy Ion Research Facility Spin spectrometer, a 4pi gamma-detector array^2. Our magnetic-substate population and angular-distribution data for single and mutual inelastic scattering suggest a spin assignment of J^pi = 36 ^+ for the resonance seen at E_ {c.m} = 45.70 MeV. Also, these data suggest a dominant decay l value of l = 34hbar for this resonance in both single and mutual inelastic scattering. The resonance spin and decay l values are 2 to 4 units above the grazing angular moment generated by optical model calculations. We used similar techniques to study the one and two alpha-transfer reactions ^{24}Mg(^ {24}Mg,^{20} Ne)^{28}Si and ^{24}Mg(^ {24}Mg,^{16} O)^{32}S. These data show that the details of these heavy-ion reactions depend critically upon the angular momentum matching properties of these different heavy-ion systems. Our results also suggest weak decay branches for these resonances to the mass-asymmetric ^{16}O + ^{32}S system. We use the Rotating Liquid Drop Model to examine the structure of the composite nucleus ^{48} Cr at high spin and excitation energy. The equilibrium shapes, energy levels and fission barriers obtained from these calculations suggest that the observed resonances correspond to the population of highly deformed, high spin states in the composite nucleus ^{48 }Cr. ftn^1R. W. Zurmuhle, et al., Phys. Lett. 129B, 384 (1983). ^2 M. Jaaskelainen, et al., Nucl. Instr. and Meth. 204, 285 (1983).

  15. Observation of Strong Resonant Behavior in the Inverse Photoelectron Spectroscopy of Ce Oxide

    SciTech Connect

    Tobin, J G; Yu, S W; Chung, B W; Waddill, G D; Damian, E; Duda, L; Nordgren, J

    2009-12-15

    X-ray Emission Spectroscopy (XES) and Resonant Inverse Photoelectron Spectroscopy (RIPES) have been used to investigate the photon emission associated with the Ce3d5/2 and Ce3d3/2 thresholds. Strong resonant behavior has been observed in the RIPES of Ce Oxide near the 5/2 and 3/2 edges. Inverse Photoelectron Spectroscopy (IPES) and its high energy variant, Bremstrahlung Isochromat Spectroscopy (BIS), are powerful techniques that permit a direct interrogation of the low-lying unoccupied electronic structure of a variety of materials. Despite being handicapped by counting rates that are approximately four orders of magnitude less that the corresponding electron spectroscopies (Photoelectron Spectroscopy, PES, and X-ray Photoelectron Spectroscopy, XPS) both IPES and BIS have a long history of important contributions. Over time, an additional variant of this technique has appeared, where the kinetic energy (KE) of the incoming electron and photon energy (hv) of the emitted electron are roughly the same magnitude as the binding energy of a core level of the material in question. Under these circumstances and in analogy to Resonant Photoelectron Spectroscopy, a cross section resonance can occur, giving rise to Resonant Inverse Photoelectron Spectroscopy or RIPES. Here, we report the observation of RIPES in an f electron system, specifically the at the 3d{sub 5/2} and 3d{sub 3/2} thresholds of Ce Oxide. The resonant behavior of the Ce4f structure at the 3d thresholds has been addressed before, including studies of the utilization of the technique as a probe of electron correlation in a variety of Ce compounds. Interestingly, the first RIPES work on rare earths dates back to 1974, although under conditions which left the state of the surface and near surface regions undefined. Although they did not use the more modern terminology of 'RIPES,' it is clear that RIPES was actually first performed in 1974 by Liefeld, Burr and Chamberlain on both La and Ce based materials. In

  16. Phase coherence of conduction electrons below the Kondo temperature

    NASA Astrophysics Data System (ADS)

    Alzoubi, Gassem M.; Birge, Norman O.

    2007-03-01

    The scattering of conduction electrons by magnetic impurities is known as the Kondo effect. This effect has been the subject of theoretical and experimental investigations for several decades. Until very recently [1, 2], however, there was no theoretical expression for the temperature dependence of the inelastic scattering rate valid for temperatures T not too far below the Kondo temperature, TK. We present experimental measurements of the phase decoherence rate, τφ-1, of conduction electrons in disordered dilute AgFe Kondo wires [3]. We compare the temperature dependence of the magnetic scattering rate, γm, with a recent theory of dephasing by Kondo impurities [2]. A good agreement with theory is obtained for T/TK > 0.1. At lower T, γm deviates from theory with a flatter T-dependence. [1] G. Zarand, L. Borda, J. von Delft, and N. Andrei, Phys.Rev. Lett. 93, 107204 (2004). [2] T. Micklitz, A. Altland, T. A. Costi, A. Rosch, Phys.Rev. Lett. 96, 226601 (2006). [3] G.M. Alzoubi and N.O. Birge, Phys.Rev. Lett. in press (2006).

  17. Manifestation of the Kondo effect in nonlinear optical absorption

    NASA Astrophysics Data System (ADS)

    Shahbazyan, T. V.; Perakis, I. E.; Raikh, M. E.

    2000-03-01

    We study the nonlinear optical absorption due to transitions from a deep impurity to states above a Fermi sea. Previous calculations(See, e.g., S. Mukamel, Principles of Nonlinear Optical Spectroscopy), (Oxford University Press, 1995). of \\chi^(3) included contributions from virtual processes involving doubly occupied impurity state. This indicates the necessity of incorporating the Hubbard repulsion of electrons at the impurity in calculation of nonlinear optical properties. Detailed calculations are performed for pump-probe spectrum. We demonstrate that Hubbard-repulsion-induced suppression of two-electron states leads to the divergency in \\chi^(3) near the absorption threshold. The origin of this divergency lies in the Kondo-physics;(See, e.g., A. C. Hewson, The Kondo Problem to Heavy Fermions), (Cambridge University Press, 1993). a monochromatic optical field induces the coupling between the impurity and conduction band states that is similar to the hybridization terms in the Anderson model.^3 Remarkably, for light-induced Kondo-absorption, the Kondo temperature can be tuned by the intensity and frequency of the pump field.

  18. Kondo effect in coupled quantum dots: A noncrossing approximation study

    NASA Astrophysics Data System (ADS)

    Aguado, Ramón; Langreth, David C.

    2003-06-01

    The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson Hamiltonian with interimpurity hopping. The Hamiltonian, formulated in slave-boson language, is solved by means of a generalization of the noncrossing approximation (NCA) to the present problem. We provide benchmark calculations of the predictions of the NCA for the linear and nonlinear transport properties of coupled quantum dots in the Kondo regime. We give a series of predictions that can be observed experimentally in linear and nonlinear transport measurements through coupled quantum dots. Importantly, it is demonstrated that measurements of the differential conductance G=dI/dV, for the appropriate values of voltages and interdot tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. This coherence can be also detected in the linear transport through the system: the curve linear conductance vs temperature is nonmonotonic, with a maximum at a temperature T* characterizing quantum coherence between both the Kondo states.

  19. Quantum quench of Kondo correlations in optical absorption

    NASA Astrophysics Data System (ADS)

    Weichselbaum, Andreas

    2013-03-01

    Absorption spectra of individual semiconductor quantum dots tunnel-coupled to a degenerate electron gas in the Kondo regime have recently become accessible to the experiment. The absorption of a single photon leads to an abrupt change in the system Hamiltonian, which can be tailored such that it results in a quantum quench of the Kondo correlations. This is accompanied by a clear signature in the form of an Anderson orthogonality catastrophe, induced by a vanishing overlap between initial and final many-body wave functions and with power-law exponents that can be tuned by an applied magnetic field. We have modeled the experiment in terms of an Anderson impurity model undergoing an optically induced quench, and studied this Kondo exciton in detail using both analytical methods and the Numerical Renormalization Group (NRG). Our NRG results reproduce the measured absorption line shapes very well, showing that NRG is ideally suited for the study of Kondo excitons. In summary, the experiments demonstrate that optical measurements on single artificial atoms offer new perspectives on many-body phenomena previously studied using transport spectroscopy only. Co-authors: Andreas Weichselbaum, Markus Hanl, and Jan von Delft, Ludwig Maximilians University.

  20. Surface Kondo effect and non-trivial metallic state of the Kondo insulator YbB12.

    PubMed

    Hagiwara, Kenta; Ohtsubo, Yoshiyuki; Matsunami, Masaharu; Ideta, Shin-Ichiro; Tanaka, Kiyohisa; Miyazaki, Hidetoshi; Rault, Julien E; Fèvre, Patrick Le; Bertran, François; Taleb-Ibrahimi, Amina; Yukawa, Ryu; Kobayashi, Masaki; Horiba, Koji; Kumigashira, Hiroshi; Sumida, Kazuki; Okuda, Taichi; Iga, Fumitoshi; Kimura, Shin-Ichi

    2016-01-01

    A synergistic effect between strong electron correlation and spin-orbit interaction has been theoretically predicted to realize new topological states of quantum matter on Kondo insulators (KIs), so-called topological Kondo insulators (TKIs). One TKI candidate has been experimentally observed on the KI SmB6(001), and the origin of the surface states (SS) and the topological order of SmB6 has been actively discussed. Here, we show a metallic SS on the clean surface of another TKI candidate YbB12(001) using angle-resolved photoelectron spectroscopy. The SS shows temperature-dependent reconstruction corresponding to the Kondo effect observed for bulk states. Despite the low-temperature insulating bulk, the reconstructed SS with c-f hybridization is metallic, forming a closed Fermi contour surrounding on the surface Brillouin zone and agreeing with the theoretically expected behaviour for SS on TKIs. These results demonstrate the temperature-dependent holistic reconstruction of two-dimensional states localized on KIs surface driven by the Kondo effect. PMID:27576449

  1. Surface Kondo effect and non-trivial metallic state of the Kondo insulator YbB12

    NASA Astrophysics Data System (ADS)

    Hagiwara, Kenta; Ohtsubo, Yoshiyuki; Matsunami, Masaharu; Ideta, Shin-Ichiro; Tanaka, Kiyohisa; Miyazaki, Hidetoshi; Rault, Julien E.; Fèvre, Patrick Le; Bertran, François; Taleb-Ibrahimi, Amina; Yukawa, Ryu; Kobayashi, Masaki; Horiba, Koji; Kumigashira, Hiroshi; Sumida, Kazuki; Okuda, Taichi; Iga, Fumitoshi; Kimura, Shin-Ichi

    2016-08-01

    A synergistic effect between strong electron correlation and spin-orbit interaction has been theoretically predicted to realize new topological states of quantum matter on Kondo insulators (KIs), so-called topological Kondo insulators (TKIs). One TKI candidate has been experimentally observed on the KI SmB6(001), and the origin of the surface states (SS) and the topological order of SmB6 has been actively discussed. Here, we show a metallic SS on the clean surface of another TKI candidate YbB12(001) using angle-resolved photoelectron spectroscopy. The SS shows temperature-dependent reconstruction corresponding to the Kondo effect observed for bulk states. Despite the low-temperature insulating bulk, the reconstructed SS with c-f hybridization is metallic, forming a closed Fermi contour surrounding on the surface Brillouin zone and agreeing with the theoretically expected behaviour for SS on TKIs. These results demonstrate the temperature-dependent holistic reconstruction of two-dimensional states localized on KIs surface driven by the Kondo effect.

  2. Modeling the nuclear magnetic resonance behavior of lung: from electrical engineering to critical care medicine.

    PubMed

    Cutillo, A G; Ailion, D C

    1999-01-01

    The present article reviews the basic principles of a new approach to the characterization of pulmonary disease. This approach is based on the unique nuclear magnetic resonance (NMR) properties of the lung and combines experimental measurements (using specially developed NMR techniques) with theoretical simulations. The NMR signal from inflated lungs decays very rapidly compared with the signal from completely collapsed (airless) lungs. This phenomenon is due to the presence of internal magnetic field inhomogeneity produced by the alveolar air-tissue interface (because air and water have different magnetic susceptibilities). The air-tissue interface effects can be detected and quantified by magnetic resonance imaging (MRI) techniques using temporally symmetric and asymmetric spin-echo sequences. Theoretical models developed to explain the internal (tissue-induced) magnetic field inhomogeneity in aerated lungs predict the NMR lung behavior as a function of various technical and physiological factors (e.g., the level of lung inflation) and simulate the effects of various lung disorders (in particular, pulmonary edema) on this behavior. Good agreement has been observed between the predictions obtained from the mathematical models and the results of experimental NMR measurements in normal and diseased lungs. Our theoretical and experimental data have important pathophysiological and clinical implications, especially with respect to the characterization of acute lung disease (e.g., pulmonary edema) and the management of critically ill patients.

  3. Kondo effect in magnetic tunnel junctions with an AlOx tunnel barrier

    NASA Astrophysics Data System (ADS)

    Zheng, Chao; Shull, Robert D.; Chen, P. J.; Pong, Philip W. T.

    2016-06-01

    The influence of the magnetization configuration on the Kondo effect in a magnetic tunnel junction is investigated. In the parallel configuration, an additional resistance contribution (R*) below 40 K exhibits a logarithmic temperature dependence, indicating the presence of the Kondo effect. However, in the anti-parallel configuration, the Kondo-effect-associated spin-flip scattering has a nontrivial contribution to the tunneling current, which compensates the reduction of the current directly caused by Kondo scattering, making R* disappear. These results indicate that suppression and restoration of the Kondo effect can be experimentally achieved by altering the magnetization configuration, enhancing our understanding of the role of the Kondo effect in spin-dependent transport.

  4. Direct evidence for suppression of the Kondo effect due to pure spin current

    NASA Astrophysics Data System (ADS)

    Hamaya, K.; Kurokawa, T.; Oki, S.; Yamada, S.; Kanashima, T.; Taniyama, T.

    2016-10-01

    We study the effect of a pure spin current on the Kondo singlet in a diluted magnetic alloy using nonlocal lateral spin valve structures with highly spin polarized Co2FeSi electrodes. Temperature dependence of the nonlocal spin signals shows a sharp reduction with decreasing temperature, followed by a plateau corresponding to the low temperature Fermi liquid regime below the Kondo temperature (TK). The spin diffusion length of the Kondo alloy is found to increase with increasing spin accumulation. The results are in agreement with the intuitive description that the Kondo singlet cannot survive any more in sufficiently large spin accumulation even below TK.

  5. Universal low-temperature crossover in two-channel Kondo models

    NASA Astrophysics Data System (ADS)

    Mitchell, Andrew K.; Sela, Eran

    2012-06-01

    An exact expression is derived for the electron Green function in two-channel Kondo models with one and two impurities, describing the crossover from non-Fermi liquid (NFL) behavior at intermediate temperatures to standard Fermi liquid (FL) physics at low temperatures. Symmetry-breaking perturbations generically present in experiment ensure the standard low-energy FL description, but the full crossover is wholly characteristic of the unstable NFL state. Distinctive conductance lineshapes in quantum dot devices should result. We exploit a connection between this crossover and one occurring in a classical boundary Ising model to calculate real-space electron densities at finite temperature. The single universal finite-temperature Green function is then extracted by inverting the integral transformation relating these Friedel oscillations to the t matrix. Excellent agreement is demonstrated between exact results and full numerical renormalization group calculations.

  6. Two-dimensional Fermi surfaces in Kondo insulator SmB₆.

    PubMed

    Li, G; Xiang, Z; Yu, F; Asaba, T; Lawson, B; Cai, P; Tinsman, C; Berkley, A; Wolgast, S; Eo, Y S; Kim, Dae-Jeong; Kurdak, C; Allen, J W; Sun, K; Chen, X H; Wang, Y Y; Fisk, Z; Li, Lu

    2014-12-01

    In the Kondo insulator samarium hexaboride (SmB6), strong correlation and band hybridization lead to an insulating gap and a diverging resistance at low temperature. The resistance divergence ends at about 3 kelvin, a behavior that may arise from surface conductance. We used torque magnetometry to resolve the Fermi surface topology in this material. The observed oscillation patterns reveal two Fermi surfaces on the (100) surface plane and one Fermi surface on the (101) surface plane. The measured Fermi surface cross sections scale as the inverse cosine function of the magnetic field tilt angles, which demonstrates the two-dimensional nature of the conducting electronic states of SmB6. PMID:25477456

  7. Resonant behavior of trapped Brownian particles in an oscillatory shear flow.

    PubMed

    Kählert, Hanno; Löwen, Hartmut

    2012-10-01

    The response of harmonically trapped Brownian particles to an externally imposed oscillatory shear flow is explored by theory and computer simulation. The special case of a single trapped particle is solved analytically. We present explicit results for the time-dependent density and the velocity distribution. The response of the many-body problem is studied by computer simulations. In particular, we investigate the influence of oscillatory shear flow on the internal modes of the cluster. As a function of the shear oscillation frequency, we find resonant behavior for certain (antisymmetric) normal modes, implying that they can be efficiently excited by oscillatory shear. Our results are verifiable in experiments on dusty plasmas and trapped colloidal dispersions.

  8. Kondo effect goes anisotropic in vanadate oxide superlattices

    NASA Astrophysics Data System (ADS)

    Rotella, H.; Pautrat, A.; Copie, O.; Boullay, P.; David, A.; Mercey, B.; Morales, M.; Prellier, W.

    2015-11-01

    We study the transport properties in SrVO3/LaVO3 (SVO/LVO) superlattices deposited on SrTiO3 (STO) substrates. We show that the electronic conduction occurs in the metallic LVO layers with a galvanomagnetism typical of a 2D Fermi surface. In addition, a Kondo-like component appears in both the thermal variation of resistivity and the magnetoresistance. Surprisingly, in this system where the STO interface does not contribute to the measured conduction, the Kondo correction is strongly anisotropic. We show that the growth temperature allows a direct control of this contribution. Finally, the key role of vanadium mixed valency stabilized by oxygen vacancies is enlightened.

  9. The Spin Glass-Kondo Competition in Disordered Cerium Systems

    NASA Astrophysics Data System (ADS)

    Magalhaes, S. G.; Zimmer, F.; Coqblin, B.

    2013-10-01

    We discuss the competition between the Kondo effect, the spin glass state and a magnetic order observed in disordered Cerium systems. We present firstly the experimental situation of disordered alloys such as CeNi1 - xCux and then the different theoretical approaches based on the Kondo lattice model, with different descriptions of the intersite exchange interaction for the spin glass. After the gaussian approach of the Sherrington-Kirkpatrick model, we discuss the Mattis and the van Hemmen models. Then, we present simple cluster calculations in order to describe the percolative evolution of the clusters from the cluster spin glass to the inhomogeneous ferromagnetic order recently observed in CeNi1 - xCux disordered alloys and finally we discuss the effect of random and transverse magnetic field.

  10. Characterization of a correlated topological Kondo insulator in one dimension

    NASA Astrophysics Data System (ADS)

    Hagymási, I.; Legeza, Ö.

    2016-04-01

    We investigate the ground state of a p -wave Kondo-Heisenberg model introduced by Alexandrov and Coleman with an Ising-type anisotropy in the Kondo interaction and correlated conduction electrons. Our aim is to understand how they affect the stability of the Haldane state obtained in the SU(2)-symmetric case without the Hubbard interaction. By applying the density-matrix renormalization group algorithm and calculating the entanglement entropy we show that in the anisotropic case a phase transition occurs and a Néel state emerges above a critical value of the Coulomb interaction. These findings are also corroborated by the examination of the entanglement spectrum and the spin profile of the system which clarify the structure of each phase.

  11. Kondo and Majorana doublet interactions in quantum dots

    NASA Astrophysics Data System (ADS)

    Kim, Younghyun; Liu, Dong E.; Gaidamauskas, Erikas; Paaske, Jens; Flensberg, Karsten; Lutchyn, Roman

    We study the properties of a quantum dot coupled to a normal lead and a time-reversal topological superconductor with Majorana Kramers pair at the end. We explore the phase diagram of the system as a function of Kondo and Majorana-induced coupling strengths using perturbative renormalization group study and slave-boson mean-field theory. We find that, in the presence of coupling between a quantum dot and a Majorana doublet, the system flows to a new fixed point controlled by the Majorana doublet, rather than the Kondo coupling, which is characterized by correlations between a localized spin and the fermion parity of each spin sector of the topological superconductor. We find that this fixed point is stable with respect to Gaussian fluctuations. We also investigate the effect of spin-spin interaction between a quantum dot and Majorana doublet and compare the result with a case where a normal lead is directly coupled to Majorana doublet.

  12. Resonances and resonance widths

    SciTech Connect

    Collins, T.

    1986-05-01

    Two-dimensional betatron resonances are much more important than their simple one-dimensional counterparts and exhibit a strong dependence on the betatron phase advance per cell. A practical definition of ''width'' is expanded upon in order to display these relations in tables. A primarily pedagogical introduction is given to explain the tables, and also to encourage a wider capability for deriving resonance behavior and wider use of ''designer'' resonances.

  13. Neutron scattering from the Kondo Insulator SmB6

    NASA Astrophysics Data System (ADS)

    Broholm, Collin

    A review of neutron scattering work probing the Kondo insulator SmB6 is presented with special emphasis on assessing the topology of the underlying strongly renormalized band structure. A 14 meV excition dominates the spectrum and is evidence of strong electron correlations [1]. Though the data generally supports the proposal that SmB6 is a topological Kondo insulator, specific heat and high-resolution neutron scattering data show a continuum of states well below the bulk transport gap, which enrich the problem and may connect to the recent surprising de Haas van Alpen results. ``Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6,'' W. T. Fuhrman, J. Leiner, P. Nikolic, G. E. Granroth, M. B. Stone, M. D. Lumsden, L. DeBeer-Schmitt, P. A. Alekseev, J.-M. Mignot, S. M. Koohpayeh, P. Cottingham, W. Adam Phelan, L. Schoop, T. M. McQueen, and C. Broholm, Phys. Rev. Lett. 114, 036401 (2015). Supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering, under Grant No. DEFG02-08ER46544 and the Gordon and Betty Moore Foundation.

  14. Kondo physics from quasiparticle poisoning in Majorana devices

    NASA Astrophysics Data System (ADS)

    Plugge, S.; Zazunov, A.; Eriksson, E.; Tsvelik, A. M.; Egger, R.

    2016-03-01

    We present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M =2 attached leads, such "dangerous" quasiparticle poisoning processes cause a spin S =1 /2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effect of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, for M >3 , the topological Kondo fixed point re-emerges, though now it involves only M -1 leads. As a consequence, for M =3 , the low-energy fixed point becomes trivial corresponding to decoupled leads.

  15. Kondo physics from quasiparticle poisoning in Majorana devices

    DOE PAGES

    Plugge, S.; Tsvelik, A. M.; Zazunov, A.; Eriksson, E.; Egger, R.

    2016-03-24

    Here, we present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M = 2 attached leads, such “dangerous” quasiparticle poisoning processes cause a spin S = 1/2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effectmore » of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, for M > 3, the topological Kondo fixed point re-emerges, though now it involves only M–1 leads. As a consequence, for M = 3, the low-energy fixed point becomes trivial corresponding to decoupled leads.« less

  16. Observation of the two-channel Kondo effect

    NASA Astrophysics Data System (ADS)

    Potok, R. M.; Rau, I. G.; Shtrikman, Hadas; Oreg, Yuval; Goldhaber-Gordon, D.

    2007-03-01

    Some of the most intriguing problems in solid-state physics arise when the motion of one electron dramatically affects the motion of surrounding electrons. Traditionally, such highly correlated electron systems have been studied mainly in materials with complex transition metal chemistry. Over the past decade, researchers have learned to confine one or a few electrons within a nanometre-scale semiconductor `artificial atom', and to understand and control this simple system in detail3. Here we combine artificial atoms to create a highly correlated electron system within a nano-engineered semiconductor structure. We tune the system in situ through a quantum phase transition between two distinct states, each a version of the Kondo state, in which a bound electron interacts with surrounding mobile electrons. The boundary between these competing Kondo states is a quantum critical point-namely, the exotic and previously elusive two-channel Kondo state, in which electrons in two reservoirs are entangled through their interaction with a single localized spin.

  17. The resonance overlap criterion and the onset of stochastic behavior in the restricted three-body problem

    NASA Technical Reports Server (NTRS)

    Wisdom, J.

    1980-01-01

    The resonance overlap criterion for the onset of stochastic behavior is applied to the planar circular-restricted three-body problem with small mass ratio (mu). Its predictions for mu = 0.001, 0.0001, and 0.00001 are compared to the transitions observed in the numerically determined Kolmogorov-Sinai entropy and found to be in remarkably good agreement. In addition, an approximate scaling law for the onset of stochastic behavior is derived.

  18. Resonant Dynamics of Grounded Cognition: Explanation of Behavioral and Neuroimaging Data Using the ART Neural Network

    PubMed Central

    Domijan, Dražen; Šetić, Mia

    2016-01-01

    Research on grounded cognition suggests that the processing of a word or concept reactivates the perceptual representations that are associated with the referent object. The objective of this work is to demonstrate how behavioral and functional neuroimaging data on grounded cognition can be understood as different manifestations of the same cortical circuit designed to achieve stable category learning, as proposed by the adaptive resonance theory (ART). We showed that the ART neural network provides a mechanistic explanation of why reaction times in behavioral studies depend on the expectation or attentional priming created by the word meaning (Richter and Zwaan, 2009). A mismatch between top-down expectation and bottom-up sensory data activates an orienting subsystem that slows execution of the current task. Furthermore, we simulated the data from functional neuroimaging studies of color knowledge retrieval that showed anterior shift (Chao and Martin, 1999; Thompson-Schill, 2003) and an overlap effect (Simmons et al., 2007; Hsu et al., 2011) in the left fusiform gyrus. We explain the anterior effect as a result of the partial activation of different components of the same ART circuit in the condition of passive viewing. Conversely, a demanding perceptual task requires activation of the whole ART circuit. This condition is reflected in the fMRI image as an overlap between cortical activation during perceptual and conceptual processing. We conclude that the ART neural network is able to explain how the brain grounds symbols in perception via perceptual simulation. PMID:26903933

  19. Effects of Nonsphericity on the Behavior of Lorenz-Mie Resonances in Scattering Characteristics of Liquid-Cloud Droplets

    NASA Technical Reports Server (NTRS)

    Dlugach, Janna M.; Mishchenko, Michael I.

    2014-01-01

    By using the results of highly accurate T-matrix computations for randomly oriented oblate and prolate spheroids and Chebyshev particles with varying degrees of asphericity, we analyze the effects of a deviation of water-droplet shapes from that of a perfect sphere on the behavior of Lorenz-Mie morphology-dependent resonances of various widths. We demonstrate that the positions and profiles of the resonances can change significantly with increasing asphericity. The absolute degree of asphericity required to suppress a Lorenz-Mie resonance is approximately proportional to the resonance width. Our results imply that numerical averaging of scattering characteristics of real cloud droplets over sizes may rely on a significantly coarser size-parameter resolution than that required for ideal, perfectly spherical particles.

  20. Two-channel Kondo effect and renormalization flow with macroscopic quantum charge states.

    PubMed

    Iftikhar, Z; Jezouin, S; Anthore, A; Gennser, U; Parmentier, F D; Cavanna, A; Pierre, F

    2015-10-01

    Many-body correlations and macroscopic quantum behaviours are fascinating condensed matter problems. A powerful test-bed for the many-body concepts and methods is the Kondo effect, which entails the coupling of a quantum impurity to a continuum of states. It is central in highly correlated systems and can be explored with tunable nanostructures. Although Kondo physics is usually associated with the hybridization of itinerant electrons with microscopic magnetic moments, theory predicts that it can arise whenever degenerate quantum states are coupled to a continuum. Here we demonstrate the previously elusive 'charge' Kondo effect in a hybrid metal-semiconductor implementation of a single-electron transistor, with a quantum pseudospin of 1/2 constituted by two degenerate macroscopic charge states of a metallic island. In contrast to other Kondo nanostructures, each conduction channel connecting the island to an electrode constitutes a distinct and fully tunable Kondo channel, thereby providing unprecedented access to the two-channel Kondo effect and a clear path to multi-channel Kondo physics. Using a weakly coupled probe, we find the renormalization flow, as temperature is reduced, of two Kondo channels competing to screen the charge pseudospin. This provides a direct view of how the predicted quantum phase transition develops across the symmetric quantum critical point. Detuning the pseudospin away from degeneracy, we demonstrate, on a fully characterized device, quantitative agreement with the predictions for the finite-temperature crossover from quantum criticality.

  1. Optical Study of Interactions in a d-Electron Kondo Lattice with Ferromagnetism

    SciTech Connect

    Burch, K. S.; Schafgans, A.; Butch, N. P.; Sayles, T. A.; Maple, M. B.; Sales, Brian C; Mandrus, David; Basov, D. N.

    2005-01-01

    We report on a comprehensive optical, transport, and thermodynamic study of the Zintl compound Yb{sub 14}MnSb{sub 11}, demonstrating that it is the first ferromagnetic Kondo lattice compound in the underscreened limit. We propose a scenario whereby the combination of Kondo and Jahn-Teller effects provides a consistent explanation of both transport and optical data.

  2. Quantum phase transitions and anomalous Hall effect in a pyrochlore Kondo lattice

    NASA Astrophysics Data System (ADS)

    Grefe, Sarah; Ding, Wenxin; Si, Qimiao

    The metallic variant of the pyrochlore iridates Pr2Ir2O7 has shown characteristics of a possible chiral spin liquid state [PRL 96 087204 (2006), PRL 98, 057203 (2007), Nature 463, 210 (2010)] and quantum criticality [Nat. Mater. 13, 356 (2014)]. An important question surrounding the significant anomalous Hall response observed in Pr2Ir2O7 is the nature of the f-electron local moments, including their Kondo coupling with the conduction d-electrons. The heavy effective mass and related thermodynamic characteristics indicate the involvement of the Kondo effect in this system's electronic properties. In this work, we study the effects of Kondo coupling on candidate time-reversal-symmetry-breaking spin liquid states on the pyrochlore lattice. Representing the f-moments as slave fermions Kondo-coupled to conduction electrons, we study the competition between Kondo-singlet formation and chiral spin correlations and determine the zero-temperature phase diagram. We derive an effective chiral interaction between the local moments and the conduction electrons and calculate the anomalous Hall response across the quantum phase transition from the Kondo destroyed phase to the Kondo screened phase. We discuss our results' implications for Pr2Ir2O7 and related frustrated Kondo-lattice systems.

  3. Fano Profiles in STM Spectroscopy of Single and Corraled Kondo Adsorbates

    NASA Astrophysics Data System (ADS)

    Gadzuk, J. W.; Plihal, M.

    2001-03-01

    Resonance tunneling STM studies of transition metal atoms adsorbed on noble metal surfaces have produced spatially-dependent differential conductance versus voltage spectra, frequently observed to be asymmetric Fano lineshapes. The basic ideas behind the Fano profile of isolated atoms have been adapted to a theory of STM spectroscopy of atoms adsorbed on surfaces. The state of the tunneling electron within an STM tip biased with respect to the surface is regarded as the initially excited state. The atom on the surface plays the role of Fano’s discrete state embedded in the continuum. The normalized differential conductivity associated with the resonance, the STM equivalent of a spectral lineshape, is described by an expression that is related to, but more complicated than the Fano formula. It also contains more information, particularly that which is relevant to electron surface transport and scattering from artificially-synthesized surface nanostructures such as quantum corrals. Theoretical temperature and tip-position-dependent tunneling characteristics for Kondo systems such as single and “corraled” Co or Ce adsorbed on Au(111) will be presented and discussed.

  4. Valley blockade and multielectron spin-valley Kondo effect in silicon

    NASA Astrophysics Data System (ADS)

    Crippa, A.; Tagliaferri, M. L. V.; Rotta, D.; De Michielis, M.; Mazzeo, G.; Fanciulli, M.; Wacquez, R.; Vinet, M.; Prati, E.

    2015-07-01

    We report on the valley blockade and the multielectron Kondo effect generated by an impurity atom in a silicon nanofield effect device. According to the spin-valley nature of tunneling processes, and consistently with those allowed by the valley blockade regime, the manifestation of Kondo effect at occupation N =1 ,2 ,3 has the periodicity 4 of the electron filling sequence typical of silicon. The spin-valley Kondo effect emerges under different kinds of screening depending on the electron filling. By exploiting the valley blockade regime, valley index conservation in the Kondo SU(4) is deduced with no need of an external magnetic field. Microwave irradiation suppresses the Kondo effect at occupancies up to three electrons.

  5. Scanning tunneling spectroscopy of a magnetic atom on graphene in the Kondo regime

    DOE PAGES

    Zhuang, Huai -Bin; Sun, Qing -feng; Xie, X. C.

    2009-06-23

    In this study, the Kondo effect in the system consisting of a magnetic adatom on the graphene is studied. By using the non-equilibrium Green function method with the slave-boson mean field approximation, the local density of state (LDOS) and the conductance are calculated. For a doped graphene, the Kondo phase is present at all time. Surprisingly, two kinds of Kondo regimes are revealed. But for the undoped graphene, the Kondo phase only exists if the adatom’s energy level is beyond a critical value. The conductance is similar to the LDOS, thus, the Kondo peak in the LDOS can be observedmore » with the scanning tunneling spectroscopy. In addition, in the presence of a direct coupling between the STM tip and the graphene, the conductance may be dramatically enhanced, depending on the coupling site.« less

  6. Scanning tunneling spectroscopy of a magnetic atom on graphene in the Kondo regime

    SciTech Connect

    Zhuang, Huai -Bin; Sun, Qing -feng; Xie, X. C.

    2009-06-23

    In this study, the Kondo effect in the system consisting of a magnetic adatom on the graphene is studied. By using the non-equilibrium Green function method with the slave-boson mean field approximation, the local density of state (LDOS) and the conductance are calculated. For a doped graphene, the Kondo phase is present at all time. Surprisingly, two kinds of Kondo regimes are revealed. But for the undoped graphene, the Kondo phase only exists if the adatom’s energy level is beyond a critical value. The conductance is similar to the LDOS, thus, the Kondo peak in the LDOS can be observed with the scanning tunneling spectroscopy. In addition, in the presence of a direct coupling between the STM tip and the graphene, the conductance may be dramatically enhanced, depending on the coupling site.

  7. Strong suppression of superconductivity by divalent ytterbium Kondo holes in CeCoIn5

    NASA Astrophysics Data System (ADS)

    Shimozawa, M.; Watashige, T.; Yasumoto, S.; Mizukami, Y.; Nakamura, M.; Shishido, H.; Goh, S. K.; Terashima, T.; Shibauchi, T.; Matsuda, Y.

    2012-10-01

    To study the nature of partially substituted Yb ions in a Ce-based Kondo lattice, we fabricated high quality Ce1-xYbxCoIn5 epitaxial thin films using molecular beam epitaxy. We find that the Yb substitution leads to a linear decrease of the unit cell volume—indicating that Yb ions are divalent, forming Kondo holes in Ce1-xYbxCoIn5—and leads to a strong suppression of the superconductivity and Kondo coherence. These results, combined with measurements of the Hall effect, indicate that Yb ions act as nonmagnetic impurity scatterers in the coherent Kondo lattice without serious suppression of the antiferromagnetic fluctuations. These results are in stark contrast to previous studies performed using bulk single crystals, which claim the importance of valence fluctuations of Yb ions. The present work also highlights the suitability of epitaxial films in the study of the impurity effect on the Kondo lattice.

  8. Fermionology in the Kondo-Heisenberg model: the case of CeCoIn5

    NASA Astrophysics Data System (ADS)

    Zhong, Yin; Zhang, Lan; Lu, Han-Tao; Luo, Hong-Gang

    2015-09-01

    The Fermi surface of heavy electron systems plays a fundamental role in understanding their variety of puzzling phenomena, for example, quantum criticality, strange metal behavior, unconventional superconductivity and even enigmatic phases with yet unknown order parameters. The spectroscopy measurement of the typical heavy fermion superconductor CeCoIn5 has demonstrated multi-Fermi surface structure, which has not been studied in detail theoretically in a model system like the Kondo-Heisenberg model. In this work, we take a step toward such a theoretical model by revisiting the Kondo-Heisenberg model. It is found that the usual self-consistent calculation cannot reproduce the fermionology of the experimental observation of the system due to the sign binding between the hopping of the conduction electrons and the mean-field valence-bond order. To overcome such inconsistency, the mean-field valence-bond order is considered as a free/fitting parameter to correlate them with real-life experiments as performed in recent experiments [M.P. Allan, F. Massee, D.K. Morr, J. Van Dyke, A.W. Rost, A.P. Mackenzie, C. Petrovic, J.C. Davis, Nat. Phys. 9, 468 (2013); J. Van Dyke, F. Massee, M.P. Allan, J.C. Davis, C. Petrovic, D.K. Morr, Proc. Natl. Acad. Sci. 111, 11663 (2014)], which also explicitly reflects the intrinsic dispersion of local electrons observed in experimental measurements. Given the fermionology, the calculated effective mass enhancement, entropy, superfluid density and Knight shift are all in qualitative agreement with the experimental results of CeCoIn5, which confirms our assumption. Our result supports a d_{x^2 - y^2 }-wave pairing structure in the heavy fermion material CeCoIn5.

  9. STEM in Kondo Lattices: a new window on correlated electron materials

    NASA Astrophysics Data System (ADS)

    Coleman, Piers

    2012-02-01

    The tremendous developments in scanning tunneling electron spectroscopy over the past decade, applied with tremendous success to the cuprate superconductors, are now beginning to be applied to other strongly correlated electron systems. One area where they offer tremendous potential, is in the context of heavy fermion materials. In the last few years, it has become possible to start probing the physics of the Kondo lattice using STEM methods. In this talk I will review this field, discussing the physics of tunneling into the Kondo lattice, showing how tunneling involves a co-operative process of electron transfer and spin-flip, called ``cotunnelling'' [1,2]. I will provide an overview of latest results in this field, especially URu2Si2 [3,4], YbRh2Si2 [5] and CeCoIn5 [6], discussing how STEM can be used to probe various new theoretical proposals [7,8] for the exotic order and critical behavior. [4pt] [1] M. Maltseva, M. Dzero, and P. Coleman, Phys. Rev. Lett. 103, 206402 (2009).[0pt] [2] J. Figgins and D. Morr, Phys. Rev. Lett. 104, 187202 (2010).[0pt] [3] A. R. Schmidt et al, Nature 465, 570-576 (2010).[0pt] [4] P. Aynajian et al., Proc. Natl. Acad. Sci. U.S.A. 107, 10383 (2010).[0pt] [5] S. Ernst et al, Nature (2011).[0pt] [6] S. Ernst et al, Physica Status Solidi 247, 624 (2010).[0pt] [7] Y. Dubi and A.V. Balatsky, Phys. Rev. Lett. 106, 196407 (2011).[0pt] [8] P. Chandra, P. Coleman and R. Flint, to be published (2012).

  10. From four- to two-channel Kondo effect in junctions of XY spin chains

    NASA Astrophysics Data System (ADS)

    Giuliano, Domenico; Sodano, Pasquale; Tagliacozzo, Arturo; Trombettoni, Andrea

    2016-08-01

    We consider the Kondo effect in Y-junctions of anisotropic XY models in an applied magnetic field along the critical lines characterized by a gapless excitation spectrum. We find that, while the boundary interaction Hamiltonian describing the junction can be recasted in the form of a four-channel, spin-1/2 antiferromagnetic Kondo Hamiltonian, the number of channels effectively participating in the Kondo effect depends on the chain parameters, as well as on the boundary couplings at the junction. The system evolves from an effective four-channel topological Kondo effect for a junction of XX-chains with symmetric boundary couplings into a two-channel one at a junction of three quantum critical Ising chains. The effective number of Kondo channels depends on the properties of the boundary and of the bulk. The XX-line is a "critical" line, where a four-channel topological Kondo effect can be recovered by fine-tuning the boundary parameter, while along the line in parameter space connecting the XX-line and the critical Ising point the junction is effectively equivalent to a two-channel topological Kondo Hamiltonian. Using a renormalization group approach, we determine the flow of the boundary couplings, which allows us to define and estimate the critical couplings and Kondo temperatures of the different Kondo (pair) channels. Finally, we study the local transverse magnetization in the center of the Y-junction, eventually arguing that it provides an effective tool to monitor the onset of the two-channel Kondo effect.

  11. Behavioral stochastic resonance associated with large-scale synchronization of human brain activity

    NASA Astrophysics Data System (ADS)

    Kitajo, Keiichi; Yamanaka, Kentaro; Nozaki, Daichi; Ward, Lawrence M.; Yamamoto, Yoshiharu

    2004-05-01

    We demonstrate experimentally that enhanced detection of weak visual signals by addition of visual noise is accompanied by an increase in phase synchronization of EEG signals across widely-separated areas of the human brain. In our sensorimotor integration task, observers responded to a weak rectangular gray-level signal presented to their right eyes by pressing and releasing a button whenever they detected an increment followed by a decrement in brightness. Signal detection performance was optimized by presenting randomly-changing-gray-level noise separately to observers' left eyes using a mirror stereoscope. We measured brain electrical activity at the scalp by electroencephalograph (EEG), calculated the instantaneous phase for each EEG signal, and evaluated the degree of large-scale phase synchronization between pairs of EEG signals. Dynamic synchronization-desynchronization patterns were observed and we found evidence of noise-enhanced large-scale synchronization associated with detection of the brightness changes under conditions of noise-enhanced performance. Our results suggest that behavioral stochastic resonance might arise from noise-enhanced synchronization of neural activities across widespread brain regions.

  12. Thermal Signatures of The Kondo Volume Collapse in Cerium

    SciTech Connect

    Lipp, M; Jackson, D; Cynn, H; Aracne, C; Evans, W; McMahan, A

    2008-05-23

    X-ray diffraction measurements of cerium in the vicinity of the isostructural {gamma}-{alpha} transition have been performed with high precision and accuracy from room temperature to almost 800 K. The disputed location of the critical point has been found to occur at 1.5 {+-} 0.1 GPa and 480 {+-} 10 K. The data is well fit by the Kondo volume collapse model plus a quasiharmonic representation of the phonons. The resultant free energy is validated against data for the thermodynamic Grueneisen parameter, and beyond the dominant spin fluctuation contribution, indicates a dramatic change in the lattice Grueneisen parameter across the transition.

  13. Beam Kondo effect? — Possible anomalous penning deexcitation spectrum

    NASA Astrophysics Data System (ADS)

    Yoshimori, A.; Makoshi, K.

    1990-05-01

    It is shown that the Penning deexcitation spectrum of the triplet 2s excited helium atom beam at metal surfaces can have a threshold anomaly, which is the Kondo effect. The time-dependent Newns-Anderson model is used to analyze the transition rate of the deexcitation in the quasi-static approximation. The effect is due to the spin as well as potential scattering of conduction electrons by the He atom in the triplet excited state as the initial state interaction. Line shape of the Penning deexcitation spectrum is discussed, and clean surfaces of alkali metals are pointed out to be possible candidates to observe this many body effect.

  14. Application of the S=1 underscreened Anderson lattice model to Kondo uranium and neptunium compounds

    NASA Astrophysics Data System (ADS)

    Thomas, Christopher; da Rosa Simões, Acirete S.; Iglesias, J. R.; Lacroix, C.; Perkins, N. B.; Coqblin, B.

    2011-01-01

    Magnetic properties of uranium and neptunium compounds showing the coexistence of the Kondo screening effect and ferromagnetic order are investigated within the Anderson lattice Hamiltonian with a two-fold degenerate f level in each site, corresponding to 5f2 electronic configuration with S=1 spins. A derivation of the Schrieffer-Wolff transformation is presented and the resulting Hamiltonian has an effective f-band term, in addition to the regular exchange Kondo interaction between the S=1 f spins and the s=1/2 spins of the conduction electrons. The resulting effective Kondo lattice model can describe both the Kondo regime and a weak delocalization of the 5f electrons. Within this model we compute the Kondo and Curie temperatures as a function of model parameters, namely the Kondo exchange interaction constant JK, the magnetic intersite exchange interaction JH, and the effective f bandwidth. We deduce, therefore, a phase diagram of the model which yields the coexistence of the Kondo effect and ferromagnetic ordering and also accounts for the pressure dependence of the Curie temperature of uranium compounds such as UTe.

  15. Kondo effect with diverging hybridization: Possible realization in graphene with vacancies

    NASA Astrophysics Data System (ADS)

    Mitchell, Andrew K.; Fritz, Lars

    2013-08-01

    We investigate Kondo physics in a host with a strongly diverging density of states. This study is motivated by a recent work on vacancies in the graphene honeycomb lattice, whose density of states is enhanced at low energies due to potential scattering. The generalized quantum impurity model describing the vacancy is shown to support a spin-(1)/(2) (doublet) Kondo phase. The special role played by a diverging host density of states is examined in detail, with distinctive signatures associated with the power law Kondo effect shown to appear in thermodynamic quantities and the scattering t matrix, with a strongly enhanced Kondo temperature. Although the effective Kondo model supports a stable phase characterized by strong renormalized particle-hole asymmetry, we find that this phase cannot in fact be accessed in the full Anderson model. In the more realistic case, where the divergence in the host density of states is cut off at low energies, a crossover is generated between pristine power law Kondo physics and a regular Kondo strong coupling state.

  16. Antiferromagnetic Kondo lattice in the layered compounds Re2NiGa9Ge2 (Re =Ce, Pr, Sm)

    NASA Astrophysics Data System (ADS)

    Zhu, Yanglin; Liu, Jinyu; Hu, Jin; Adams, Daniel; Spinu, Leonard; Mao, Zhiqiang

    Intermetallic compounds containing rare-earth/actinide elements with 4f/5f electrons have formed a special family of strongly correlated materials, i.e. heavy fermion systems. We have recently found a new layered rare earth intermetallic system showing moderate heavy fermion behavior: Re2NiGa9Ge2 (Re =Ce, Sm, Pr). The Re =Ce and Sm members were previously synthesized, while their electronic properties have not been reported. We have recently grown single crystals of Re2NiGa9Ge2 (Re =Ce, Sm, Pr) and characterized their electronic and magnetic properties. We find all these materials are antiferromagnetic, with TN = 2.5 K, 5 K, 3.4 K respectively for Re =Ce, Pr and Sm. Moreover, they also exhibit large values of electronic specific coefficient: γ ~ 101 mJ mol-Ce-1 K-2 for Re =Ce, 368 mJ mol-Pr-1 K-2 for Re =Pr, and 196.4 mJ mol-Sm-1 K-2 for Re =Sm, indicating enhanced Kondo effect and the presence of AFM Kondo lattice. Our findings suggest that Re2NiGa9Ge2 (Re =Ce, Pr, Sm) could be interesting candidate materials for exploring novel exotic properties of correlated electrons through external parameter tuning such as chemical substitution and pressure.

  17. Kondo physics in a rare earth ion with well localized 4f electrons.

    PubMed

    Stankiewicz, Jolanta; Evangelisti, Marco; Fisk, Zachary; Schlottmann, Pedro; Gor'kov, Lev P

    2012-06-22

    Dilute Nd in simple cubic LaB(6) shows electrical resistance and specific heat features at low temperature consistent with a Kondo scale of T(K) Kondo coupled to the conduction electrons in LaB(6). We conjecture that the unexpected Kondo effect arises via participation of 4f quadrupolar degrees of freedom of the Nd crystal-field, ground-state quartet.

  18. Tunable Pseudogap Kondo Effect and Quantum Phase Transitions in Aharonov-Bohm Interferometers

    SciTech Connect

    Dias Da Silva, Luis G; Sandler, Nancy; Simon, Pascal; Ingersent, Kevin; Ulloa, Sergio E

    2009-01-01

    We study two quantum dots embedded in the arms of an Aharonov-Bohm ring threaded by a magnetic flux. This system can be described by an effective one-impurity Anderson model with an energy- and flux- dependent density of states. For specific values of the flux, this density of states vanishes at the Fermi energy, yielding a controlled realization of the pseudogap Kondo effect. The conductance and trans- mission phase shifts reflect a nontrivial interplay between wave interference and interactions, providing clear signatures of quantum phase transitions between Kondo and non-Kondo ground states.

  19. Surface plasmon resonances behavior in visible light of non-metal perovskite oxides AgNbO{sub 3}

    SciTech Connect

    Zhou, Fei; Zhu, Jingchuan Liu, Yong; Zhao, Xiaoliang; Lai, Zhonghong

    2014-12-08

    We investigate the surface plasmon resonances (SPRs) behavior of silver niobate (AgNbO{sub 3}) experimentally and theoretically. Result shows that the localized SPRs (LSPRs) of AgNbO{sub 3} combining with its interband transitions enlarge the absorption band across the whole ultraviolet-visible range. The LSPRs behavior in visible-light is mainly ascribed to the metal-like state of silver ion and self-assembled microstructures of AgNbO{sub 3} microcrystal. The ab initio density functional theory calculations are carried out to obtain the further insight of the SPRs behaviors. Theoretical study indicates that the Ag atoms are weakly bound in the perovskite structure, leading to a metal-like state, which was the key factor to SPRs behavior of AgNbO{sub 3}.

  20. Cancer cell uptake behavior of Au nanoring and its localized surface plasmon resonance induced cell inactivation

    NASA Astrophysics Data System (ADS)

    Chu, Che-Kuan; Tu, Yi-Chou; Chang, Yu-Wei; Chu, Chih-Ken; Chen, Shih-Yang; Chi, Ting-Ta; Kiang, Yean-Woei; Yang, Chih-Chung

    2015-02-01

    Au nanorings (NRIs), which have the localized surface plasmon resonance (LSPR) wavelength around 1058 nm, either with or without linked antibodies, are applied to SAS oral cancer cells for cell inactivation through the LSPR-induced photothermal effect when they are illuminated by a laser of 1065 nm in wavelength. Different incubation times of cells with Au NRIs are considered for observing the variations of cell uptake efficiency of Au NRI and the threshold laser intensity for cell inactivation. In each case of incubation time, the cell sample is washed for evaluating the total Au NRI number per cell adsorbed and internalized by the cells based on inductively coupled plasma mass spectrometry measurement. Also, the Au NRIs remaining on cell membrane are etched with KI/I2 solution to evaluate the internalized Au NRI number per cell. The threshold laser intensities for cell inactivation before washout, after washout, and after KI/I2 etching are calibrated from the circular area sizes of inactivated cells around the illuminated laser spot center with various laser power levels. By using Au NRIs with antibodies, the internalized Au NRI number per cell increases monotonically with incubation time up to 24 h. However, the number of Au NRI remaining on cell membrane reaches a maximum at 12 h in incubation time. The cell uptake behavior of an Au NRI without antibodies is similar to that with antibodies except that the uptake NRI number is significantly smaller and the incubation time for the maximum NRI number remaining on cell membrane is delayed to 20 h. By comparing the threshold laser intensities before and after KI/I2 etching, it is found that the Au NRIs remaining on cell membrane cause more effective cancer cell inactivation, when compared with the internalized Au NRIs.

  1. Alveolar air-tissue interface and nuclear magnetic resonance behavior of the lung

    NASA Astrophysics Data System (ADS)

    Cutillo, Antonio G.; Ailion, David C.; Ganesan, Krishnamurthy; Morris, Alan H.; Durney, Carl H.

    1995-05-01

    The nuclear magnetic resonance (NMR) properties of lung are markedly affected by the alveolar air-tissue interface, which produces internal magnetic field inhomogeneity because of the different magnetic susceptibilities of air and water. This internal magnetic field inhomogeneity results in a marked shortening of the free induction decay (FID) (in the time domain) and in inhomogeneous NMR line broadening (in the frequency domain). The signal loss due to internal magnetic field inhomogeneity can be measured as the difference Δ between the spin-echo signals obtained using temporally symmetric and asymmetric spin-echo sequences; the degree of asymmetry of the asymmetric sequence is characterized by the asymmetry time τa. In accordance with predictions based on the analysis of theoretical models, experiments in excised rat lungs (studied at various inflation levels) have shown that Δ depends on τa and is very low in degassed lungs. When measured at τa equals 6 ms, the difference signal (Δ6ms) increases markedly with alveolar opening but does not vary significantly during the rest of the inflation-deflation cycle. In edematous (oleic acid-injured) lungs, the values of Δ6ms measured at low inflation levels are significantly below those observed in normal lungs. These results suggest that Δ6ms is very sensitive to alveolar recruitment and relatively insensitive to alveolar distension. Therefore, measurements of Δ6ms may provide a means of assessing the relative contributions of these two factors to the pressure-volume behavior of lung. Such measurements may contribute to the characterization of pulmonary edema (for example, by detecting the loss of alveolar air-tissue interface due to alveolar flooding, by differentiating interstitial from alveolar pulmonary edema, and by assessing the effects of positive airway pressures). NMR lineshape measurements can also provide valuable information regarding lung geometry and the characterization of pulmonary edema.

  2. Cancer cell uptake behavior of Au nanoring and its localized surface plasmon resonance induced cell inactivation.

    PubMed

    Chu, Che-Kuan; Tu, Yi-Chou; Chang, Yu-Wei; Chu, Chih-Ken; Chen, Shih-Yang; Chi, Ting-Ta; Kiang, Yean-Woei; Yang, Chih-Chung

    2015-02-20

    Au nanorings (NRIs), which have the localized surface plasmon resonance (LSPR) wavelength around 1058 nm, either with or without linked antibodies, are applied to SAS oral cancer cells for cell inactivation through the LSPR-induced photothermal effect when they are illuminated by a laser of 1065 nm in wavelength. Different incubation times of cells with Au NRIs are considered for observing the variations of cell uptake efficiency of Au NRI and the threshold laser intensity for cell inactivation. In each case of incubation time, the cell sample is washed for evaluating the total Au NRI number per cell adsorbed and internalized by the cells based on inductively coupled plasma mass spectrometry measurement. Also, the Au NRIs remaining on cell membrane are etched with KI/I2 solution to evaluate the internalized Au NRI number per cell. The threshold laser intensities for cell inactivation before washout, after washout, and after KI/I2 etching are calibrated from the circular area sizes of inactivated cells around the illuminated laser spot center with various laser power levels. By using Au NRIs with antibodies, the internalized Au NRI number per cell increases monotonically with incubation time up to 24 h. However, the number of Au NRI remaining on cell membrane reaches a maximum at 12 h in incubation time. The cell uptake behavior of an Au NRI without antibodies is similar to that with antibodies except that the uptake NRI number is significantly smaller and the incubation time for the maximum NRI number remaining on cell membrane is delayed to 20 h. By comparing the threshold laser intensities before and after KI/I2 etching, it is found that the Au NRIs remaining on cell membrane cause more effective cancer cell inactivation, when compared with the internalized Au NRIs.

  3. Quantum phase transitions in the Kondo-necklace model

    NASA Astrophysics Data System (ADS)

    Ghassemi, Nader; Hemmatiyan, Shayan; Rahimi Movassagh, Mahsa; Kargarian, Mahdi; Rezakhani, Ali T.; Langari, Abdollah

    2015-03-01

    Kondo-necklace model can describe the magnetic low-energy limit of strongly correlated heavy fermion materials. There exist multiple energy scales in this model corresponding to each phase of the system. Here, we study quantum phase transitions between these different phases, and show the effect of anisotropies in terms of quantum information properties and vanishing energy gap. We employ the perturbative unitary transformations to calculate the energy gap and spin-spin correlations for the model one, two, and three spatial dimensions as well as for the spin ladders. In particular, we show that the method, although being perturbative, can predict the expected quantum critical point by imposing the spontaneous symmetry breaking, which is in good agreement with the results of numerical and Green's function analyses. We also use concurrence, a bipartite entanglement measure, to study the criticality of the model. Absence of singularities in the derivative of the concurrence in 2d and 3d in Kondo-necklace model shows this model has multipartite entanglement. We also discuss the crossover from the one-dimensional to the two-dimensional model via the ladder structure. Sharif University of Technology.

  4. Phase diagram of the bosonic Kondo-Hubbard model

    SciTech Connect

    Foss-Feig, Michael; Rey, Ana Maria

    2011-11-15

    We study a bosonic version of the Kondo lattice model with an onsite repulsion in the conduction band, implemented with alkali-metal atoms in two bands of an optical lattice. Using both weak- and strong-coupling perturbation theory, we find that at unit filling of the conduction bosons the superfluid-to-Mott-insulator transition should be accompanied by a magnetic transition from a ferromagnet (in the superfluid) to a paramagnet (in the Mott insulator). Furthermore, an analytic treatment of Gutzwiller mean-field theory reveals that quantum spin fluctuations induced by the Kondo exchange cause the otherwise continuous superfluid-to-Mott-insulator phase transition to be first order. We show that lattice separability imposes a serious constraint on proposals to exploit excited bands for quantum simulations, and discuss a way to overcome this constraint in the context of our model by using an experimentally realized nonseparable lattice. A method to probe the first-order nature of the transition based on collapses and revivals of the matter-wave field is also discussed.

  5. Kondo route to spin inhomogeneities in the honeycomb Kitaev model

    NASA Astrophysics Data System (ADS)

    Das, S. D.; Dhochak, K.; Tripathi, V.

    2016-07-01

    Paramagnetic impurities in a quantum spin liquid give rise to Kondo effects with highly unusual properties. We have studied the effect of locally coupling a paramagnetic impurity with the spin-1/2 honeycomb Kitaev model in its gapless spin-liquid phase. The (impurity) scaling equations are found to be insensitive to the sign of the coupling. The weak and strong coupling fixed points are stable, with the latter corresponding to a noninteracting vacancy and an interacting, spin-1 defect for the antiferromagnetic and ferromagnetic cases, respectively. The ground state in the strong coupling limit in both cases has a nontrivial topology associated with a finite Z2 flux at the impurity site. For the antiferromagnetic case, this result has been obtained straightforwardly owing to the integrability of the Kitaev model with a vacancy. The strong-coupling limit of the ferromagnetic case is, however, nonintegrable, and we address this problem through exact-diagonalization calculations with finite Kitaev fragments. Our exact diagonalization calculations indicate that the weak-to-strong coupling transition and the topological phase transition occur rather close to each other and are possibly coincident. We also find an intriguing similarity between the magnetic response of the defect and the impurity susceptibility in the two-channel Kondo problem.

  6. Nonlinear vibration behavior of graphene resonators and their applications in sensitive mass detection

    PubMed Central

    2012-01-01

    Graphene has received significant attention due to its excellent mechanical properties, which has resulted in the emergence of graphene-based nano-electro-mechanical system such as nanoresonators. The nonlinear vibration of a graphene resonator and its application to mass sensing (based on nonlinear oscillation) have been poorly studied, although a graphene resonator is able to easily reach the nonlinear vibration. In this work, we have studied the nonlinear vibration of a graphene resonator driven by a geometric nonlinear effect due to an edge-clamped boundary condition using a continuum elastic model such as a plate model. We have shown that an in-plane tension can play a role in modulating the nonlinearity of a resonance for a graphene. It has been found that the detection sensitivity of a graphene resonator can be improved by using nonlinear vibration induced by an actuation force-driven geometric nonlinear effect. It is also shown that an in-plane tension can control the detection sensitivity of a graphene resonator that operates both harmonic and nonlinear oscillation regimes. Our study suggests the design principles of a graphene resonator as a mass sensor for developing a novel detection scheme using graphene-based nonlinear oscillators. PMID:22947221

  7. Magnetic-field-modulated Kondo effect in a single-magnetic-ion molecule

    NASA Astrophysics Data System (ADS)

    Romero, Javier I.; Vernek, E.; Martins, G. B.; Mucciolo, E. R.

    2014-11-01

    We study numerically the low-temperature electronic transport properties of a single-ion magnet with uniaxial and transverse spin anisotropies. We find clear signatures of a Kondo effect caused by the presence of a transverse (zero-field) anisotropy in the molecule. This Kondo effect has an SU(2) pseudospin character, associated with a doublet ground state of the isolated molecule, which results from the transverse anisotropy. Upon applying a transverse magnetic field to the single-ion magnet, we observe oscillations of the Kondo effect due to the presence of diabolical points (degeneracies) of the energy spectrum of the molecule caused by geometrical phase interference effects, similar to those observed in the quantum tunneling of multi-ion molecular nanomagnets. The field-induced lifting of the ground-state degeneracy competes with the interference modulation, resulting in some cases in a suppression of the Kondo peak.

  8. Surface-State Spin Textures and Mirror Chern Numbers in Topological Kondo Insulators.

    PubMed

    Legner, Markus; Rüegg, Andreas; Sigrist, Manfred

    2015-10-01

    The recent discovery of topological Kondo insulators has triggered renewed interest in the well-known Kondo insulator samarium hexaboride, which is hypothesized to belong to this family. In this Letter, we study the spin texture of the topologically protected surface states in such a topological Kondo insulator. In particular, we derive close relationships between (i) the form of the hybridization matrix at certain high-symmetry points, (ii) the mirror Chern numbers of the system, and (iii) the observable spin texture of the topological surface states. In this way, a robust classification of topological Kondo insulators and their surface-state spin texture is achieved. We underpin our findings with numerical calculations of several simplified and realistic models for systems like samarium hexaboride.

  9. The Kondo temperature of a two-dimensional electron gas with Rashba spin-orbit coupling.

    PubMed

    Chen, Liang; Sun, Jinhua; Tang, Ho-Kin; Lin, Hai-Qing

    2016-10-01

    We use the Hirsch-Fye quantum Monte Carlo method to study the single magnetic impurity problem in a two-dimensional electron gas with Rashba spin-orbit coupling. We calculate the spin susceptibility for various values of spin-orbit coupling, Hubbard interaction, and chemical potential. The Kondo temperatures for different parameters are estimated by fitting the universal curves of spin susceptibility. We find that the Kondo temperature is almost a linear function of Rashba spin-orbit energy when the chemical potential is close to the edge of the conduction band. When the chemical potential is far away from the band edge, the Kondo temperature is independent of the spin-orbit coupling. These results demonstrate that, for single impurity problems in this system, the most important reason to change the Kondo temperature is the divergence of density of states near the band edge, and the divergence is induced by the Rashba spin-orbit coupling.

  10. Probing the Kondo lattice model with alkaline-earth-metal atoms

    SciTech Connect

    Foss-Feig, Michael; Hermele, Michael; Rey, Ana Maria

    2010-05-15

    We study transport properties of alkaline-earth-metal atoms governed by the Kondo lattice Hamiltonian plus a harmonic confining potential, and suggest simple dynamical probes of several different regimes of the phase diagram that can be implemented with current experimental techniques. In particular, we show how Kondo physics at strong coupling, at low density, and in the heavy fermion phase is manifest in the dipole oscillations of the conduction band upon displacement of the trap center.

  11. Fractionalized Fermi liquid on the surface of a topological Kondo insulator

    NASA Astrophysics Data System (ADS)

    Thomson, Alex; Sachdev, Subir

    2016-03-01

    We argue that topological Kondo insulators can also have "intrinsic" topological order associated with fractionalized excitations on their surfaces. The hybridization between the local moments and conduction electrons can weaken near the surface, and this enables the local moments to form spin liquids. This coexists with the conduction electron surface states, realizing a surface fractionalized Fermi liquid. We present mean-field solutions of a Kondo-Heisenberg model in two spatial dimensions which display such surfaces.

  12. Surface morphologies, electronic structures, and Kondo effect of lanthanide(III)-phthalocyanine molecules on Au(111) by using STM, STS and FET properties for next generation devices.

    PubMed

    Katoh, Keiichi; Komeda, Tadahiro; Yamashita, Masahiro

    2010-05-28

    The crystal structures of double-decker single-molecule magnets (SMMs) LnPc(2) (Ln = Tb(III) and Dy(III); Pc = phthalocyanine) and non-SMM YPc(2) were determined by using single crystal X-ray diffraction analysis. The compounds are isomorphous to each other. The compounds have metal-centers (M(3+) = Tb, Dy, and Y) sandwiched by two Pc ligands via eight isoindole-nitrogen atoms in a square-antiprism fashion. The twist angle between the two Pc ligands is 41.4 degrees. Scanning tunneling microscopy (STM) was used to investigate the compounds adsorbed on a Au(111) surface, deposited by using thermal evaporation in ultra-high vacuum. Both MPc(2) with eight-lobes and MPc with four-lobes, which has lost one Pc ligand, were observed. In the scanning tunneling spectroscopy (STS) images of TbPc molecules at 4.8 K, a Kondo peak with a Kondo temperature (T(K)) of approximately 250 K was observed near the Fermi level (V = 0 V). On the other hand, DyPc, YPc and MPc(2) exhibited no Kondo peak. In order to understand the observed Kondo effect, the energy splitting of sublevels in a crystal field should be taken into consideration. As the next step in our studies on the SMM/Kondo effect in Tb-Pc derivatives, we investigated the electronic transport properties of Ln-Pc molecules as the active layer in top- and bottom-contact thin-film organic field effect transistor (OFETs) devices. Tb-Pc molecule devices exhibit p-type semiconducting properties with a hole mobility (mu(H)) of approximately 10(-4) cm(2) V(-1) s(-1). Interestingly, the Dy-Pc based devices exhibited ambipolar semiconducting properties with an electron mobility (mu(e)) of approximately 10(-5) and a hole mobility (mu(H)) of approximately 10(-4) cm(2) V(-1) s(-1). This behavior has important implications for the electronic structure of the molecules. PMID:20396817

  13. Local susceptibility and Kondo scaling in the presence of finite bandwidth

    NASA Astrophysics Data System (ADS)

    Hanl, Markus; Weichselbaum, Andreas

    2014-02-01

    The Kondo scale TK for impurity systems is expected to guarantee universal scaling of physical quantities. However, in practice, not every definition of TK necessarily supports this notion away from the strict scaling limit. Specifically, this paper addresses the role of finite bandwidth D in the strongly correlated Kondo regime. For this, various theoretical definitions of TK are analyzed based on the inverse magnetic impurity susceptibility at zero temperature. While conventional definitions in that respect quickly fail to ensure universal Kondo scaling for a large range of D, this paper proposes an altered definition of TKsc that allows universal scaling of dynamical or thermal quantities for a given fixed Hamiltonian. If the scaling is performed with respect to an external parameter that directly enters the Hamiltonian, such as magnetic field, the corresponding TKsc,B for universal scaling differs, yet becomes equivalent to TKsc in the scaling limit. The only requirement for universal scaling in the full Kondo parameter regime with a residual error of less than 1% is a well-defined isolated Kondo feature with TK≲0.01D irrespective of specific other impurity parameter settings. By varying D over a wide range relative to the bare energies of the impurity, for example, this allows a smooth transition from the Anderson to the Kondo model.

  14. One-dimensional Kondo lattice model at quarter filling

    NASA Astrophysics Data System (ADS)

    Xavier, J. C.; Miranda, E.

    2008-10-01

    We revisit the problem of the quarter-filled one-dimensional Kondo lattice model, for which the existence of a dimerized phase and a nonzero charge gap had been reported by Xavier [Phys. Rev. Lett. 90, 247204 (2003)]. Recently, some objections were raised claiming that the system is neither dimerized nor has a charge gap. In the interest of clarifying this important issue, we show that these objections are based on results obtained under conditions in which the dimer order is artificially suppressed. We use the incontrovertible dimerized phase of the Majumdar-Ghosh point of the J1-J2 Heisenberg model as a paradigm with which to illustrate this artificial suppression. Finally, by means of extremely accurate density-matrix renormalization-group calculations, we show that the charge gap is indeed nonzero in the dimerized phase.

  15. Anomalous Hall effect on the surface of topological Kondo insulators

    NASA Astrophysics Data System (ADS)

    König, E. J.; Ostrovsky, P. M.; Dzero, M.; Levchenko, A.

    2016-07-01

    We calculate the anomalous Hall conductivity σx y of the surface states in cubic topological Kondo insulators. We consider a generic model for the surface states with three Dirac cones on the (001) surface. The Fermi velocity, the Fermi momentum, and the Zeeman energy in different Dirac pockets may be unequal. The microscopic impurity potential mediates mixed intra- and interband extrinsic scattering processes. Our calculation of σx y is based on the Kubo-Streda diagrammatic approach. It includes diffractive skew scattering contributions originating from the rare two-impurity complexes. Remarkably, these contributions yield anomalous Hall conductivity that is independent of impurity concentration, and thus is of the same order as other known extrinsic side jump and skew scattering terms. We discuss various special cases of our results and the experimental relevance of our study in the context of the recent hysteretic magnetotransport data in SmB6 samples.

  16. Fractionalized Fermi liquid in a Kondo-Heisenberg model

    NASA Astrophysics Data System (ADS)

    Tsvelik, A. M.

    2016-10-01

    The Kondo-Heisenberg model is used as a controllable tool to demonstrate the existence of a peculiar metallic state with unbroken translational symmetry where the Fermi surface volume is not controlled by the total electron density. I use a nonperturbative approach where the strongest interactions are taken into account by means of exact solution, and corrections are controllable. In agreement with the general requirements formulated by T. Senthil et al. [Phys. Rev. Lett. 90, 216403 (2003), 10.1103/PhysRevLett.90.216403], the resulting metallic state represents a fractionalized Fermi liquid where well defined quasiparticles coexist with gapped fractionalized collective excitations. The system undergoes a phase transition to an ordered phase (charge density wave or superconducting), at the transition temperature which is parametrically small in comparison to the quasiparticle Fermi energy.

  17. Sensitivity and temperature behavior of a novel z-axis differential resonant micro accelerometer

    NASA Astrophysics Data System (ADS)

    Comi, C.; Corigliano, A.; Langfelder, G.; Zega, V.; Zerbini, S.

    2016-03-01

    The present work concerns the operating principle and a thorough experimental characterization of a new polysilicon resonant micro accelerometer for out-of-plane measurements, fabricated using an industrial surface micromachining technique. This device is characterized by differential resonant sensing, obtained from the variation of the electrostatic stiffness of two torsional resonators under the application of an external acceleration. The sensitivity, defined as the differential shift in resonance frequencies per gravity unit (lg  =  9.8 m s-2), is of about 10 Hz g-1when operated at a DC bias of 1.5 V only. Over an acceleration range larger than 10 g, the deviation from linearity is lower than 1% and the cross-axis rejection is larger than 34 dB. The resonators temperature coefficients of frequency, in the order of  -29 ppm {{}\\circ} C-1, are matched within about 0.1%, resulting in linear offset drifts against temperature lower than 5 mg up to 95 {{}\\circ} C in absence of any digital compensation.

  18. Kondo effect in Co{sub x}Cu{sub 1-x} granular alloys prepared by chemical reduction method

    SciTech Connect

    Dhara, Susmita Chowdhury, Rajeswari Roy; Bandyopadhyay, Bilwadal

    2015-06-24

    Nanostructured CoCu granular alloys Co{sub x}Cu{sub 1-x} (x ≤ 0.3) have been prepared by chemical reduction method using NaBH{sub 4} as a reducing agent. Electronic transport properties are studied in the temperature range 4-300 K. Resistance exhibits a metallic behavior below room temperature and draws a minimum near 20 K in all the samples except in Co{sub 0.3}Cu{sub 0.7}. This low temperature resistivity minimum diminishes with applied magnetic field. There is also a logarithmic temperature dependence of resistivity at temperatures below 20 K. This phenomenon indicates a Kondo-like scattering mechanism involving magnetic Co impurity spin clusters in Cu host.

  19. Topological surface states in Kondo insulator SmB6 via planar tunneling spectroscopy*

    NASA Astrophysics Data System (ADS)

    Park, Wan Kyu; Sun, Lunan; Noddings, Alex; Greene, Laura; Kim, Dae-Jeong; Fisk, Zachary

    Samarium hexaboride (SmB6) belongs to a class of materials called Kondo insulators in which the hybridization between itinerant electrons and local moments leads to an emergent state of matter. With inherently large spin-orbit coupling along with strong correlation, SmB6 has been recently predicted to be topological meaning that topologically robust conducting states should exist at its surfaces. Although extensive investigations have provided growing evidence for the existence of such states, corroborative spectroscopic evidences are still lacking unlike in the weakly correlated counterparts. We adopt planar tunneling spectroscopy to unveil their detailed nature and behavior utilizing its inherently high energy resolution. Measurements of tunneling conductance on two different crystal surfaces (001) and (011) reveal the expected linear density of states for two and one Dirac cones, respectively. Moreover, it is found that these topological states cease to be protected well before they merge into the bulk states at the gap edges. Microscopic modeling of the tunneling processes accounting for the interaction with spin excitons as predicted by a recent theory provide consistent explanations for all the observed features, corroborating the proposed picture on the incompletely protected surface states in SmB6

  20. Nonlinear dynamic behaviors of clamped laminated shallow shells with one-to-one internal resonance

    NASA Astrophysics Data System (ADS)

    Abe, Akira; Kobayashi, Yukinori; Yamada, Gen

    2007-07-01

    This paper investigates one-to-one internal resonance of laminated shallow shells with rigidly clamped edges. It is assumed that the natural frequencies ω2 and ω3 of two asymmetric (second and third) vibration modes have the relationship ω2≈ ω3. The displacements are expressed by using eigenvectors for linear vibration modes calculated by the Ritz method. Applying Galerkin's procedure to the equation of motion, nonlinear differential equations are derived. By considering the first vibration mode in addition to the two asymmetric vibration modes, quadratic nonlinear terms expressing the interaction between the asymmetric and the first modes appear in the differential equations. Shooting method is used to obtain the steady-state response when the driving frequency Ω is near ω2. The dynamic characteristics of the shells with the internal resonance are discussed.

  1. Influence of the Basset force on the resonant behavior of an oscillator with fluctuating frequency

    SciTech Connect

    Rekker, A. Mankin, R.

    2015-10-28

    The influence of hydrodynamic interactions, such as Stokes and Basset forces, on the dynamics of a harmonically trapped Brownian tracer is considered. A generalized Langevin equation is used to describe the tracer’s response to an external periodic force and to dichotomous fluctuations of the stiffness of the trapping potential. Relying on the Shapiro-Loginov formula, exact expressions for the complex susceptibility and for the response function are presented. On the basis of these exact formulas, it is demonstrated that interplay of a multiplicative colored noise and the Basset force induced memory effects can generate a variety of cooperation effects, such as multiresonance versus the driving frequency, as well as stochastic resonance versus noise parameters. In particular, in certain parameter regions the response function exhibits a resonance-like enhancement at intermediate values of the intensity of the Basset force. Conditions for the appearance of these effects are also discussed.

  2. Magnetization dynamics and ferromagnetic resonance behavior of melt spun FeBSiGe amorphous alloys

    NASA Astrophysics Data System (ADS)

    Estévez, D. C.; Betancourt, I.; Montiel, H.

    2012-09-01

    Frequency-dependent magnetic properties of melt spun Fe80B10Si10-xGex (x = 0.0-10.0) were studied by means of inductance spectroscopy (using the complex permeability formalism) and ferromagnetic resonance techniques. The magnetization dynamics showed two magnetization mechanisms, reversible bulging of domains and hysteresis. The dominant mechanism changed as Ge progressively replaced Si; the changes reflect the crystallization processes observed for higher Ge contents, x > 5. High relaxation frequencies (above 1 MHz) were observed for alloys with x ≥ 2.5. In the ferromagnetic resonance response, coupling and decoupling between the amorphous and crystalline phases were detected depending on the orientation of the alloy samples. This allowed the calculation of the anisotropy fields of the alloys—the decreasing trend with increasing Ge content was interpreted in terms of a variable easy direction.

  3. Influence of the Basset force on the resonant behavior of an oscillator with fluctuating frequency

    NASA Astrophysics Data System (ADS)

    Rekker, A.; Mankin, R.

    2015-10-01

    The influence of hydrodynamic interactions, such as Stokes and Basset forces, on the dynamics of a harmonically trapped Brownian tracer is considered. A generalized Langevin equation is used to describe the tracer's response to an external periodic force and to dichotomous fluctuations of the stiffness of the trapping potential. Relying on the Shapiro-Loginov formula, exact expressions for the complex susceptibility and for the response function are presented. On the basis of these exact formulas, it is demonstrated that interplay of a multiplicative colored noise and the Basset force induced memory effects can generate a variety of cooperation effects, such as multiresonance versus the driving frequency, as well as stochastic resonance versus noise parameters. In particular, in certain parameter regions the response function exhibits a resonance-like enhancement at intermediate values of the intensity of the Basset force. Conditions for the appearance of these effects are also discussed.

  4. If It's Resonance, What is Resonating?

    ERIC Educational Resources Information Center

    Kerber, Robert C.

    2006-01-01

    The phenomenon under the name "resonance," which, is based on the mathematical analogy between mechanical resonance and the behavior of wave functions in quantum mechanical exchange phenomena was described. The resonating system does not have a structure intermediate between those involved in the resonance, but instead a structure which is further…

  5. Magnetic moments and non-Fermi-liquid behavior in quasicrystals

    NASA Astrophysics Data System (ADS)

    Andrade, Eric

    Motivated by the intrinsic non-Fermi-liquid behavior observed in the heavy-fermion quasicrystal Au51Al34Yb15, we study the low-temperature behavior of dilute magnetic impurities placed in metallic quasicrystals. We find that a large fraction of the magnetic moments are not quenched down to very low temperatures, leading to a power-law distribution of Kondo temperatures, accompanied by a non-Fermi-liquid behavior, in a remarkable similarity to the Kondo-disorder scenario found in disordered heavy-fermion metals. This work was supported by FAPESP (Brazil) Grant No. 2013/00681-8.

  6. Verilog-A behavioral model for resonance-modulated silicon micro-ring modulator.

    PubMed

    Rhim, Jinsoo; Ban, Yoojin; Yu, Byung-Min; Lee, Jeong-Min; Choi, Woo-Young

    2015-04-01

    We present an accurate behavior model for Si micro-ring modulators (MRM) based on Verilog-A, a standard simulation tool for electronic system design. Our model describes the electrical characteristics of the Si MRM using an equivalent circuit and the optical characteristics based on the couple-mode theory. The accuracy of our model is confirmed by comparing simulation results of our behavior model with the measurement results of a fabricated Si MRM. With this behavior model, co-simulation of Si MRM and electronic driving circuits in the standard electronic design environment can be easily performed.

  7. Exploring the phase diagram of the two-impurity Kondo problem

    PubMed Central

    Spinelli, A.; Gerrits, M.; Toskovic, R.; Bryant, B.; Ternes, M.; Otte, A. F.

    2015-01-01

    A system of two exchange-coupled Kondo impurities in a magnetic field gives rise to a rich phase space hosting a multitude of correlated phenomena. Magnetic atoms on surfaces probed through scanning tunnelling microscopy provide an excellent platform to investigate coupled impurities, but typical high Kondo temperatures prevent field-dependent studies from being performed, rendering large parts of the phase space inaccessible. We present a study of pairs of Co atoms on insulating Cu2N/Cu(100), which each have a Kondo temperature of only 2.6 K. The pairs are designed to have interaction strengths similar to the Kondo temperature. By applying a sufficiently strong magnetic field, we are able to access a new phase in which the two coupled impurities are simultaneously screened. Comparison of differential conductance spectra taken on the atoms to simulated curves, calculated using a third-order transport model, allows us to independently determine the degree of Kondo screening in each phase. PMID:26616044

  8. Study of ultrasonic attenuation for the Kondo and magnetic effects in heavy fermion systems

    NASA Astrophysics Data System (ADS)

    Baral, Purna Chandra; Rout, Govind Chandra

    2013-05-01

    The heavy fermion (HF) systems draw considerable attention due to their cooperative phenomena and anomalous properties arising out of the huge effective mass. A heavy fermion system is described by a model Hamiltonian consisting of the Kondo lattice model in addition to the Heisenberg-type spin-spin interaction among the localised electrons. The Hamiltonian is treated in the mean-field approximation to find the Kondo singlet parameter λ and the short-ranged f-electron correlation parameter Γ. In order to investigate ultrasonic absorption in the system, we consider the phonon interaction with the bare f-electrons, and the phonon coupling to the Kondo singlets. Further, the phonon Hamiltonian is considered in the harmonic approximation. The phonon Green's function is calculated in closed form. The imaginary part of the phonon self-energy describes the ultrasonic attenuation for the HF systems. The calculated ultrasonic attenuation clearly displays the f-electron correlation region separated by the Kondo singlet state at low temperatures. The correlation transition temperature and the Kondo temperature are located at dips in the temperature-dependent ultrasonic attenuation. The parameter dependence of the attenuation is investigated by varying the physical parameters of the HF systems and the wave frequency, and the experimental observations are explained on the basis of the model calculations.

  9. Orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films

    DOE PAGES

    Zhu, L. J.; Nie, S. H.; Xiong, P.; Schlottmann, P.; Zhao, J. H.

    2016-02-24

    The orbital two-channel Kondo effect displaying exotic non-Fermi liquid behaviour arises in the intricate scenario of two conduction electrons compensating a pseudo-spin-1/2 impurity of two-level system. Despite extensive efforts for several decades, no material system has been clearly identified to exhibit all three transport regimes characteristic of the two-channel Kondo effect in the same sample, leaving the interpretation of the experimental results a subject of debate. Here we present a transport study suggestive of a robust orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films, as evidenced by a magnetic field-independent resistivity upturn with a clear transition from logarithmic- tomore » square-root temperature dependence and deviation from it in three distinct temperature regimes. Lastly, our results also provide an experimental indication of the presence of two-channel Kondo physics in a ferromagnet, pointing to considerable robustness of the orbital two-channel Kondo effect even in the presence of spin polarization of the conduction electrons.« less

  10. Replica symmetry breaking in a quantum spin glass-antiferromagnetic Kondo lattice

    NASA Astrophysics Data System (ADS)

    Magalhaes, S. G.; Zimmer, F. M.; Coqblin, B.

    2008-04-01

    The competition between the Kondo effect and the glassy magnetic order has been studied in a theoretical model of a Kondo lattice with an intrasite Kondo interaction. The spin glass (SG) and the antiferromagnetic (AF) orderings are described by two Kondo sublattices with infinite-range Ising SG interactions among localized spins and the disordered interactions can occur with spins of same sublattices and between spins of distinct sublattices. A transverse field Γ is introduced in the effective model as a quantum mechanism to produce spin flipping. The problem is formulated in a Grassmann path integral formalism. The disorder is treated within the replica trick in one-step replica symmetry breaking (1S-RSB). The static ansatz is adopted to get a mean-field expression for the free energy and order parameters. Results show a transition from the AF order to an RSB region with a finite staggered magnetization (mixed phase) when temperature T decreases for low values of the Kondo interaction. The SG phase is not observed below the mixed phase for 1S-RSB solution, in contrast with previous replica symmetry (RS) results. The Γ field suppresses the Neel temperature leading it to a quantum critical point.

  11. Ferromagnetism in the Kondo-lattice compound CePd2P2.

    PubMed

    Tran, Vinh Hung; Bukowski, Zbigniew

    2014-06-25

    We report physical properties of CePd2P2 crystallizing in the tetragonal ThCr2Si2-type structure (space group I4/mmm). Dc-magnetic susceptibility, magnetization, specific heat, electrical resistivity and magnetoresistance measurements establish a ferromagnetic ordering below the Curie temperature TC = 28.4 ± 0.2 K. Critical analysis of isothermal and isofield magnetization yields critical exponents of β = 0.405 ± 0.005, γ = 1.11 ± 0.05 and δ = 3.74 ± 0.04. The ordered state is characterized by saturation moment Ms ∼ 0.98μB and magnon energy gap Δ/kB ∼25–35 K. The studied properties reflect a competing influence of the Kondo and crystalline electric field (CEF) interactions. The strength of the Kondo effect is assigned by a low-temperature Kondo scale TK ∼19 ± 10 K and a high-temperature Kondo scale TK ~ H 117 } 10 K. A model of the inelastic scattering of the conduction electrons with an exchanged CEF energy ΔCEF was applied to the magnetic resistivity. An average value ΔCEF = 260 ± 30 K is consistent in the relationships with TK and TK H. We argue that the CePd2P2 compound appears to be a new ferromagnetic Kondo-lattice among the Ce-based intermetallics.

  12. Orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films

    PubMed Central

    Zhu, L. J.; Nie, S. H.; Xiong, P.; Schlottmann, P.; Zhao, J. H.

    2016-01-01

    The orbital two-channel Kondo effect displaying exotic non-Fermi liquid behaviour arises in the intricate scenario of two conduction electrons compensating a pseudo-spin-1/2 impurity of two-level system. Despite extensive efforts for several decades, no material system has been clearly identified to exhibit all three transport regimes characteristic of the two-channel Kondo effect in the same sample, leaving the interpretation of the experimental results a subject of debate. Here we present a transport study suggestive of a robust orbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films, as evidenced by a magnetic field-independent resistivity upturn with a clear transition from logarithmic- to square-root temperature dependence and deviation from it in three distinct temperature regimes. Our results also provide an experimental indication of the presence of two-channel Kondo physics in a ferromagnet, pointing to considerable robustness of the orbital two-channel Kondo effect even in the presence of spin polarization of the conduction electrons. PMID:26905518

  13. First-principles study of the Kondo physics of a single Pu impurity in a Th host

    DOE PAGES

    Zhu, Jian -Xin; Albers, R. C.; Haule, K.; Wills, J. M.

    2015-04-23

    Based on its condensed-matter properties, crystal structure, and metallurgy, which includes a phase diagram with six allotropic phases, plutonium is one of the most complicated pure elements in its solid state. Its anomalous properties, which are indicative of a very strongly correlated state, are related to its special position in the periodic table, which is at the boundary between the light actinides that have itinerant 5f electrons and the heavy actinides that have localized 5f electrons. As a foundational study to probe the role of local electronic correlations in Pu, we use the local-density approximation together with a continuous-time quantummore » Monte Carlo simulation to investigate the electronic structure of a single Pu atom that is either substitutionally embedded in the bulk and or adsorbed on the surface of a Th host. This is a simpler case than the solid phases of Pu metal. With the Pu impurity atom we have found a Kondo resonance peak, which is an important signature of electronic correlations, in the local density of states around the Fermi energy. We show that the peak width of this resonance is narrower for Pu atoms at the surface of Th than for those in the bulk due to a weakened Pu - 5f hybridization with the ligands at the surface.« less

  14. First-principles study of the Kondo physics of a single Pu impurity in a Th host

    SciTech Connect

    Zhu, Jian -Xin; Albers, R. C.; Haule, K.; Wills, J. M.

    2015-04-23

    Based on its condensed-matter properties, crystal structure, and metallurgy, which includes a phase diagram with six allotropic phases, plutonium is one of the most complicated pure elements in its solid state. Its anomalous properties, which are indicative of a very strongly correlated state, are related to its special position in the periodic table, which is at the boundary between the light actinides that have itinerant 5f electrons and the heavy actinides that have localized 5f electrons. As a foundational study to probe the role of local electronic correlations in Pu, we use the local-density approximation together with a continuous-time quantum Monte Carlo simulation to investigate the electronic structure of a single Pu atom that is either substitutionally embedded in the bulk and or adsorbed on the surface of a Th host. This is a simpler case than the solid phases of Pu metal. With the Pu impurity atom we have found a Kondo resonance peak, which is an important signature of electronic correlations, in the local density of states around the Fermi energy. We show that the peak width of this resonance is narrower for Pu atoms at the surface of Th than for those in the bulk due to a weakened Pu - 5f hybridization with the ligands at the surface.

  15. First-principles study of the Kondo physics of a single Pu impurity in a Th host

    NASA Astrophysics Data System (ADS)

    Zhu, Jian-Xin; Albers, R. C.; Haule, K.; Wills, J. M.

    2015-04-01

    Based on its condensed-matter properties, crystal structure, and metallurgy, which includes a phase diagram with six allotropic phases, plutonium is one of the most complicated pure elements in its solid state. Its anomalous properties, which are indicative of a very strongly correlated state, are related to its special position in the periodic table, which is at the boundary between the light actinides that have itinerant 5 f electrons and the heavy actinides that have localized 5 f electrons. As a foundational study to probe the role of local electronic correlations in Pu, we use the local-density approximation together with a continuous-time quantum Monte Carlo simulation to investigate the electronic structure of a single Pu atom that is either substitutionally embedded in the bulk and or adsorbed on the surface of a Th host. This is a simpler case than the solid phases of Pu metal. For the Pu impurity atom we have found a Kondo resonance peak, which is an important signature of electronic correlations, in the local density of states around the Fermi energy. Furthermore, we show that the peak width of this resonance is narrower for Pu atoms at the surface of Th than for those in the bulk due to a weakened Pu -5 f hybridization with the ligands at the surface.

  16. Transport Spectroscopy of Coupled Quantum Dots in Conditions of the Kondo Effect

    NASA Astrophysics Data System (ADS)

    Glazman, Leonid

    2005-03-01

    We develop electron transport theory for novel devices [1,2], which are interesting in the context of correlated electrons physics. The device proposed in Ref. [1] is designed for an observation of a non-Fermi-liquid behavior of itinerant electrons. The device measured in Ref. [2] may serve a similar purpose, and also may become important for quantum computing.In the case of Ref. [1], our theory [3] provides a strategy for tuning to the non-Fermi-liquid fixed point -- a quantum critical point in the space of device parameters. We explore the corresponding quantum phase transition, and make explicit predictions for the behavior of differential conductance in the vicinity of the quantum critical point. Motivated by the measurements [2], we developed a theory of conductance of Kondo quantum dots coupled by the RKKY interaction [4]. Investigation of the differential conductance at fixed interaction strength may allow one to distinguish between the possible ground states of the system. Transition between the ground states is achieved by tuning the interaction strength; the nature of the transition (which includes a possibility of a non-Fermi-liquid point) can be extracted from the temperature dependence of the linear conductance.This research is supported by NSF grants DMR02-37296 and EIA02- 10736.1. Y. Oreg and D. Goldhaber-Gordon, Phys. Rev. Lett. 90, p. 136602 (2003). 2. N.J. Craig J.M. Taylor, E.A. Lester, C.M. Marcus, M.P. Hanson, and A.C. Gossard, Science 304, 565 (2004).3. M.G. Vavilov and L.I. Glazman, preprint cond-mat/0404366.4. M. Pustilnik, L. Borda, L.I. Glazman, and J. von Delft, Phys. Rev. B 69, 115316 (2004).

  17. Ultraviolet resonance Raman and absorption difference spectroscopy of myoglobins: titration behavior of individual tyrosine residues.

    PubMed

    Asher, S A; Larkin, P J; Teraoka, J

    1991-06-18

    The UV resonance Raman spectra of horse and sperm whale myoglobin excited at 240 nm show bands between 600 and 1700 cm-1 which derive from tyrosyl and tryptophyl residues. No significant contribution from phenylalanine and peptide backbone vibrations occurs at this excitation wavelength. We examine the pH dependence of the UV resonance Raman and UV absorption difference spectra of these myoglobins to correlate the local protein environment of the tyrosyl residues as given by the protein crystal structure to their pKa values, molar absorptivities, and Raman cross sections. Some of our pKa values for the tyrosinate residues of horse Mb differ from those of previous studies. We show that the lambda max values, the molar absorptivities, and the Raman cross sections are sensitive to the local environment of the tyrosinate residues in the protein. We relate differences in the tyrosyl absorption spectra to differences in Raman cross sections. In addition, we discuss the importance to the Raman cross sections of the local electromagnetic field enhancement due to the dielectric environment of the tyrosinate residues in the protein. This local field should scale the Raman cross sections in a way useful as a probe of the average aromatic amino acid residue environment.

  18. Two-channel orbital Kondo effect in a quantum dot with SO(n) symmetry

    NASA Astrophysics Data System (ADS)

    Kuzmenko, T.; Kikoin, K.; Avishai, Y.

    2013-09-01

    A scenario for the formation of non-Fermi-liquid (NFL) Kondo effect (KE) with spin variable enumerating Kondo channels is suggested and worked out. In a doubly occupied symmetric triple quantum dot within parallel geometry, the NFL low-energy regime arises provided the device possesses both source-drain and left-right parity. Kondo screening follows a multistage renormalization group mechanism: reduction of the energy scale is accompanied by the change of the relevant symmetry group from SO(8) to SO(5). At low energy, three phases compete: (1) an underscreening spin-triplet (conventional) KE, (2) a spin-singlet potential scattering, and (3) a NFL phase where the roles of spin and orbital degrees of freedom are swapped.

  19. Spin- and angle-resolved photoemission on the topological Kondo insulator candidate: SmB6.

    PubMed

    Xu, Nan; Ding, Hong; Shi, Ming

    2016-09-14

    Topological Kondo insulators are a new class of topological insulators in which metallic surface states protected by topological invariants reside in the bulk band gap at low temperatures. Unlike other 3D topological insulators, a truly insulating bulk state, which is critical for potential applications in next-generation electronic devices, is guaranteed by many-body effects in the topological Kondo insulator. Furthermore, the system has strong electron correlations that can serve as a testbed for interacting topological theories. This topical review focuses on recent advances in the study of SmB6, the most promising candidate for a topological Kondo insulator, from the perspective of spin- and angle-resolved photoemission spectroscopy with highlights of some important transport results.

  20. Kondo effects in a triangular triple quantum dot II: ground-state properties for deformed configurations

    NASA Astrophysics Data System (ADS)

    Oguri, Akira; Amaha, Shinichi; Nisikawa, Yunori; Hewson, A. C.; Tarucha, Seigo; Numata, Takahide

    2010-03-01

    We study transport through a triangular triple quantum dot (TTQD) connected to two noninteracting leads, using the numerical renormalization group. The system has been theoretically revealed to show a variety of Kondo effects depending on the electron filling of the triangle [1]. For instance, the SU(4) Kondo effect takes place at three-electron filling, and a two-stage Kondo screening of a high-spin S=1 Nagaoka state takes place at four-electron filling. Because of the enhanced freedom in the configurations, however, the large parameter space of the TTQD still has not been fully explored, especially for large deformations. We report the effects of the inhomogeneity in the inter-dot couplings and the level positions in a wide region of the filling. [1] T. Numata, Y. Nisikawa, A. Oguri, and A. C. Hewson: PRB 80, 155330 (2009).

  1. Spin- and angle-resolved photoemission on the topological Kondo insulator candidate: SmB6

    NASA Astrophysics Data System (ADS)

    Xu, Nan; Ding, Hong; Shi, Ming

    2016-09-01

    Topological Kondo insulators are a new class of topological insulators in which metallic surface states protected by topological invariants reside in the bulk band gap at low temperatures. Unlike other 3D topological insulators, a truly insulating bulk state, which is critical for potential applications in next-generation electronic devices, is guaranteed by many-body effects in the topological Kondo insulator. Furthermore, the system has strong electron correlations that can serve as a testbed for interacting topological theories. This topical review focuses on recent advances in the study of SmB6, the most promising candidate for a topological Kondo insulator, from the perspective of spin- and angle-resolved photoemission spectroscopy with highlights of some important transport results.

  2. Kondo-type transport through a quantum dot under magnetic fields

    SciTech Connect

    Dong, Bing; Lei, X. L.

    2001-06-15

    In this paper, we investigate the Kondo correlation effects on linear and nonlinear transport in a quantum dot connected to reservoirs under finite magnetic fields, using the slave-boson mean field approach suggested by Kotliar and Ruckenstein [Phys. Rev. Lett. >57, 1362 (1986)]. A brief comparison between the present formulation and other slave-boson formulation is presented to justify this approach. The numerical results show that the linear conductance near electron-hole symmetry is suppressed by the application of the magnetic fields, but an anomalous enhancement is predicted in the nonsymmetry regime. The effect of external magnetic fields on the nonlinear differential conductances is discussed for the Kondo system. A significant reduction of the peak splitting is observed due to the strong Kondo correlation, which agrees well with experimental data.

  3. Kondo hole route to incoherence in the periodic Anderson model

    NASA Astrophysics Data System (ADS)

    Kumar, Pramod; Vidhyadhiraja, N. S.

    2013-03-01

    The interplay of disorder and interactions in strongly correlated electronic systems is a subject of perennial interest. In this work, we have investigated the effect of Kondo-hole type disorder on the dynamics and transport properties of heavy fermion systems. We employ the periodic Anderson model within the framework of coherent potential approximation and dynamical mean field theory. The crossover from lattice coherent behaviour to an incoherent single-impurity behaviour is reflected in all aspects: a highly frequency (ω)-dependent hybridization becomes almost flat, the coherence peak in resistivity (per impurity) gives way to a Hammann form that saturates at low temperature (T); the Drude peak and the mid-infrared peak in the optical conductivity vanish almost completely. The zero temperature resistivity can be captured in a closed form expression, and we show how the Nordheim's rule gets strongly modified in these systems. The thermopower exhibits a characteristic peak, which changes sign with increasing disorder, and its location is shown to correspond to the low energy scale of the system (ωL). In fact, the thermopower appears to be much more sensitive to disorder variations than the resistivity. A comparison to experiments yields quantitative agreement. JNCASR and CSIR

  4. ESR (electron spin resonance)-determined osmotic behavior of bull spermatozoa

    SciTech Connect

    Du, J.; Kleinhans, F.W.; Spitzer, V.J.; Critser, J.K. . Dept. of Medical Research); Horstman, L. . School of Veterinary Medicine); Mazur, P. )

    1990-01-01

    Our laboratories are pursuing a fundamental approach to the problems of semen cryopreservation. For many cell types (human red cells, yeast, HeLa) it has been demonstrated that there is an optimum cooling rate for cryopreservation. Faster rates allow insufficient time for cell dehydration and result in intracellular ice formation and cell death. It is possible to predict this optimal rate provided that the cell acts as an ideal osmometer and several other cell parameters are known such as the membrane hydraulic conductivity. It is the purpose of this work to examine the osmotic response of bull sperm to sucrose and NaCl utilizing electron spin resonance (ESR) to measure cell volume. For calibration purposes we also measured the ESR response of human red cells (RBC), the osmotic response of which is well documented with other methods. 15 refs., 1 fig.

  5. Charge Kondo anomalies in PbTe doped with Tl impurities.

    PubMed

    Costi, T A; Zlatić, V

    2012-01-20

    We investigate the properties of PbTe doped with a small concentration x of Tl impurities acting as acceptors and described by Anderson impurities with negative onsite correlation energy. We use the numerical renormalization group method to show that the resulting charge Kondo effect naturally accounts for the unusual low temperature and doping dependence of normal state properties, including the self-compensation effect in the carrier density and the nonmagnetic Kondo anomaly in the resistivity. These are found to be in good qualitative agreement with experiment. Our results for the Tl s-electron spectral function provide a new interpretation of point contact data.

  6. Magnetoresistance in the Spin-Orbit Kondo State of Elemental Bismuth

    PubMed Central

    Craco, Luis; Leoni, Stefano

    2015-01-01

    Materials with strong spin-orbit coupling, which competes with other particle-particle interactions and external perturbations, offer a promising route to explore novel phases of quantum matter. Using LDA + DMFT we reveal the complex interplay between local, multi-orbital Coulomb and spin-orbit interaction in elemental bismuth. Our theory quantifies the role played by collective dynamical fluctuations in the spin-orbit Kondo state. The correlated electronic structure we derive is promising in the sense that it leads to results that might explain why moderate magnetic fields can generate Dirac valleys and directional-selective magnetoresistance responses within spin-orbit Kondo metals. PMID:26358556

  7. Observation of the Kondo effect in a spin-3/2 hole quantum dot

    SciTech Connect

    Klochan, O.; Micolich, A. P.; Hamilton, A. R.; Trunov, K.; Reuter, D.; Wieck, A. D.

    2013-12-04

    We report the observation of the Kondo effect in a spin-3/2 hole quantum dot formed near pinch-off in a GaAs quantum wire. We clearly observe two distinctive hallmarks of quantum dot Kondo physics. First, the zero-bias peak in the differential conductance splits an in-plane magnetic field and the splitting is independent of gate voltage. Second, the splitting rate is twice as large as that for the lowest one-dimensional subband. We show that the Zeeman splitting of the zero-bias peak is highly anisotropic and attribute this to the strong spin-orbit interaction for holes in GaAs.

  8. Displacement and resonance behaviors of a piezoelectric diaphragm driven by a double-sided spiral electrode

    NASA Astrophysics Data System (ADS)

    Shen, Zhiyuan; Olfatnia, Mohammad; Miao, Jianmin; Wang, Zhihong

    2012-05-01

    This paper presents the design of a lead zirconate titanate (PZT) diaphragm actuated by double-sided patterned electrodes. Au/Cr electrodes were deposited on bulk PZT wafers by sputtering while patterned by a lift-off process. SU-8 thick film was used to form the structural layer. Double-spiral electrode induced in-plane poling and piezoelectric elongation are converted to an out-of-plane displacement due to the confined boundary condition. The influence of different drive configurations and electrode parameters on deflection has been calculated by finite element methods (FEM) using a uniform field model. Impedance and quasi-static displacement spectra of the diaphragm were measured after poling. A double-sided patterned electrode diaphragm can be actuated by more drive configurations than a single-sided one. Compared with a single-sided electrode drive, a double-sided out-of-phase drive configuration increases the coupling coefficient of the fundamental resonance from 7.6% to 11.8%. The displacement response of the diaphragm increases from 2.6 to 8.6 nm V-1. Configurations including the electric field component perpendicular to the poling direction can stimulate shear modes of the diaphragm.

  9. Antiferromagnetic Kondo lattice in the layered compound CePd1–xBi₂ and comparison to the superconductor LaPd1–xBi₂

    DOE PAGES

    Han, Fei; Wan, Xiangang; Phelan, Daniel; Stoumpos, Constantinos C.; Sturza, Mihai; Malliakas, Christos D.; Li, Qing'an; Han, Tian-Heng; Zhao, Qingbiao; Chung, Duck Young; et al

    2015-07-13

    The layered compound CePd1–xBi₂ with the tetragonal ZrCuSi₂-type structure was obtained from excess Bi flux. Magnetic susceptibility data of CePd1–xBi₂ show an antiferromagnetic ordering below 6 K and are anisotropic along the c axis and the ab plane. The anisotropy is attributed to crystal-electric-field (CEF) effects and a CEF model which is able to describe the susceptibility data is given. An enhanced Sommerfeld coefficient γ of 0.191 J mol Ce⁻¹ K⁻² obtained from specific-heat measurement suggests a moderate Kondo effect in CePd1–xBi₂. Other than the antiferromagnetic peak at 6 K, the resistivity curve shows a shoulderlike behavior around 75 Kmore » which could be attributed to the interplay between Kondo and CEF effects. Magnetoresistance and Hall-effect measurements suggest that the interplay reconstructs the Fermi-surface topology of CePd1–xBi₂ around 75 K. Electronic structure calculations reveal that the Pd vacancies are important to the magnetic structure and enhance the CEF effects which quench the orbital moment of Ce at low temperatures.« less

  10. Behavioral, blood, and magnetic resonance imaging biomarkers of experimental mild traumatic brain injury.

    PubMed

    Wright, David K; Trezise, Jack; Kamnaksh, Alaa; Bekdash, Ramsey; Johnston, Leigh A; Ordidge, Roger; Semple, Bridgette D; Gardner, Andrew J; Stanwell, Peter; O'Brien, Terence J; Agoston, Denes V; Shultz, Sandy R

    2016-01-01

    Repeated mild traumatic brain injuries (mTBI) may lead to serious neurological consequences, especially if re-injury occurs within the period of increased cerebral vulnerability (ICV) triggered by the initial insult. MRI and blood proteomics might provide objective measures of pathophysiological changes in mTBI, and indicate when the brain is no longer in a state of ICV. This study assessed behavioral, MRI, and blood-based markers in a rat model of mTBI. Rats were given a sham or mild fluid percussion injury (mFPI), and behavioral testing, MRI, and blood collections were conducted up to 30 days post-injury. There were cognitive impairments for three days post-mFPI, before normalizing by day 5 post-injury. In contrast, advanced MRI (i.e., tractography) and blood proteomics (i.e., vascular endothelial growth factor) detected a number of abnormalities, some of which were still present 30 days post-mFPI. These findings suggest that MRI and blood proteomics are sensitive measures of the molecular and subtle structural changes following mTBI. Of particular significance, this study identified novel tractography measures that are able to detect mTBI and may be more sensitive than traditional diffusion-tensor measures. Furthermore, the blood and MRI findings may have important implications in understanding ICV and are translatable to the clinical setting. PMID:27349514

  11. Behavioral, blood, and magnetic resonance imaging biomarkers of experimental mild traumatic brain injury

    PubMed Central

    Wright, David K.; Trezise, Jack; Kamnaksh, Alaa; Bekdash, Ramsey; Johnston, Leigh A.; Ordidge, Roger; Semple, Bridgette D.; Gardner, Andrew J.; Stanwell, Peter; O’Brien, Terence J.; Agoston, Denes V.; Shultz, Sandy R.

    2016-01-01

    Repeated mild traumatic brain injuries (mTBI) may lead to serious neurological consequences, especially if re-injury occurs within the period of increased cerebral vulnerability (ICV) triggered by the initial insult. MRI and blood proteomics might provide objective measures of pathophysiological changes in mTBI, and indicate when the brain is no longer in a state of ICV. This study assessed behavioral, MRI, and blood-based markers in a rat model of mTBI. Rats were given a sham or mild fluid percussion injury (mFPI), and behavioral testing, MRI, and blood collections were conducted up to 30 days post-injury. There were cognitive impairments for three days post-mFPI, before normalizing by day 5 post-injury. In contrast, advanced MRI (i.e., tractography) and blood proteomics (i.e., vascular endothelial growth factor) detected a number of abnormalities, some of which were still present 30 days post-mFPI. These findings suggest that MRI and blood proteomics are sensitive measures of the molecular and subtle structural changes following mTBI. Of particular significance, this study identified novel tractography measures that are able to detect mTBI and may be more sensitive than traditional diffusion-tensor measures. Furthermore, the blood and MRI findings may have important implications in understanding ICV and are translatable to the clinical setting. PMID:27349514

  12. Unconstrained muscle-tendon workloops indicate resonance tuning as a mechanism for elastic limb behavior during terrestrial locomotion.

    PubMed

    Robertson, Benjamin D; Sawicki, Gregory S

    2015-10-27

    In terrestrial locomotion, there is a missing link between observed spring-like limb mechanics and the physiological systems driving their emergence. Previous modeling and experimental studies of bouncing gait (e.g., walking, running, hopping) identified muscle-tendon interactions that cycle large amounts of energy in series tendon as a source of elastic limb behavior. The neural, biomechanical, and environmental origins of these tuned mechanics, however, have remained elusive. To examine the dynamic interplay between these factors, we developed an experimental platform comprised of a feedback-controlled servo-motor coupled to a biological muscle-tendon. Our novel motor controller mimicked in vivo inertial/gravitational loading experienced by muscles during terrestrial locomotion, and rhythmic patterns of muscle activation were applied via stimulation of intact nerve. This approach was based on classical workloop studies, but avoided predetermined patterns of muscle strain and activation-constraints not imposed during real-world locomotion. Our unconstrained approach to position control allowed observation of emergent muscle-tendon mechanics resulting from dynamic interaction of neural control, active muscle, and system material/inertial properties. This study demonstrated that, despite the complex nonlinear nature of musculotendon systems, cyclic muscle contractions at the passive natural frequency of the underlying biomechanical system yielded maximal forces and fractions of mechanical work recovered from previously stored elastic energy in series-compliant tissues. By matching movement frequency to the natural frequency of the passive biomechanical system (i.e., resonance tuning), muscle-tendon interactions resulting in spring-like behavior emerged naturally, without closed-loop neural control. This conceptual framework may explain the basis for elastic limb behavior during terrestrial locomotion. PMID:26460038

  13. Unconstrained muscle-tendon workloops indicate resonance tuning as a mechanism for elastic limb behavior during terrestrial locomotion.

    PubMed

    Robertson, Benjamin D; Sawicki, Gregory S

    2015-10-27

    In terrestrial locomotion, there is a missing link between observed spring-like limb mechanics and the physiological systems driving their emergence. Previous modeling and experimental studies of bouncing gait (e.g., walking, running, hopping) identified muscle-tendon interactions that cycle large amounts of energy in series tendon as a source of elastic limb behavior. The neural, biomechanical, and environmental origins of these tuned mechanics, however, have remained elusive. To examine the dynamic interplay between these factors, we developed an experimental platform comprised of a feedback-controlled servo-motor coupled to a biological muscle-tendon. Our novel motor controller mimicked in vivo inertial/gravitational loading experienced by muscles during terrestrial locomotion, and rhythmic patterns of muscle activation were applied via stimulation of intact nerve. This approach was based on classical workloop studies, but avoided predetermined patterns of muscle strain and activation-constraints not imposed during real-world locomotion. Our unconstrained approach to position control allowed observation of emergent muscle-tendon mechanics resulting from dynamic interaction of neural control, active muscle, and system material/inertial properties. This study demonstrated that, despite the complex nonlinear nature of musculotendon systems, cyclic muscle contractions at the passive natural frequency of the underlying biomechanical system yielded maximal forces and fractions of mechanical work recovered from previously stored elastic energy in series-compliant tissues. By matching movement frequency to the natural frequency of the passive biomechanical system (i.e., resonance tuning), muscle-tendon interactions resulting in spring-like behavior emerged naturally, without closed-loop neural control. This conceptual framework may explain the basis for elastic limb behavior during terrestrial locomotion.

  14. Unconstrained muscle-tendon workloops indicate resonance tuning as a mechanism for elastic limb behavior during terrestrial locomotion

    PubMed Central

    Robertson, Benjamin D.; Sawicki, Gregory S.

    2015-01-01

    In terrestrial locomotion, there is a missing link between observed spring-like limb mechanics and the physiological systems driving their emergence. Previous modeling and experimental studies of bouncing gait (e.g., walking, running, hopping) identified muscle-tendon interactions that cycle large amounts of energy in series tendon as a source of elastic limb behavior. The neural, biomechanical, and environmental origins of these tuned mechanics, however, have remained elusive. To examine the dynamic interplay between these factors, we developed an experimental platform comprised of a feedback-controlled servo-motor coupled to a biological muscle-tendon. Our novel motor controller mimicked in vivo inertial/gravitational loading experienced by muscles during terrestrial locomotion, and rhythmic patterns of muscle activation were applied via stimulation of intact nerve. This approach was based on classical workloop studies, but avoided predetermined patterns of muscle strain and activation—constraints not imposed during real-world locomotion. Our unconstrained approach to position control allowed observation of emergent muscle-tendon mechanics resulting from dynamic interaction of neural control, active muscle, and system material/inertial properties. This study demonstrated that, despite the complex nonlinear nature of musculotendon systems, cyclic muscle contractions at the passive natural frequency of the underlying biomechanical system yielded maximal forces and fractions of mechanical work recovered from previously stored elastic energy in series-compliant tissues. By matching movement frequency to the natural frequency of the passive biomechanical system (i.e., resonance tuning), muscle-tendon interactions resulting in spring-like behavior emerged naturally, without closed-loop neural control. This conceptual framework may explain the basis for elastic limb behavior during terrestrial locomotion. PMID:26460038

  15. Competition between Quadrupole and Magnetic Kondo Effects in Non-Kramers Doublet Systems

    NASA Astrophysics Data System (ADS)

    Kusunose, Hiroaki; Onimaru, Takahiro

    2015-03-01

    We discuss possible competition between magnetic and quadrupole Kondo effects in non-Kramers doublet systems in cubic symmetry. The quadrupole Kondo effect leads to non-Fermi-liquid (NFL) ground state, while the magnetic one favors ordinary Fermi-liquid (FL) ground state. In terms of the j-j coupling scheme, we argue that the orbital fluctuation must develop in the vicinity of the NFL-FL boundary. A change of temperature dependence of the f-electron entropy in both the FL and NFL regimes is demonstrated by the Wilson's numerical renormalization-group (NRG) method on the basis of the extended two-channel Kondo exchange model. We present implications to PrT2X20 (T=Ti, V, Ir; X=Al, Zn) systems which exhibit both quadrupole ordering and peculiar superconductivity. We discuss how the magnetic field lifts the non-Kramers degeneracy. Our model also represents the alternative FL state accompanied by a free magnetic spin, as a consequence of stronger competition between the magnetic and the quadrupole Kondo effects.

  16. Quantum phase transitions, frustration, and the Fermi surface in the Kondo lattice model

    NASA Astrophysics Data System (ADS)

    Eidelstein, Eitan; Moukouri, S.; Schiller, Avraham

    2011-07-01

    The quantum phase transition from a spin-Peierls phase with a small Fermi surface to a paramagnetic Luttinger-liquid phase with a large Fermi surface is studied in the framework of a one-dimensional Kondo-Heisenberg model that consists of an electron gas away from half filling, coupled to a spin-1/2 chain by Kondo interactions. The Kondo spins are further coupled to each other with isotropic nearest-neighbor and next-nearest-neighbor antiferromagnetic Heisenberg interactions which are tuned to the Majumdar-Ghosh point. Focusing on three-eighths filling and using the density-matrix renormalization-group (DMRG) method, we show that the zero-temperature transition between the phases with small and large Fermi momenta appears continuous, and involves a new intermediate phase where the Fermi surface is not well defined. The intermediate phase is spin gapped and has Kondo-spin correlations that show incommensurate modulations. Our results appear incompatible with the local picture for the quantum phase transition in heavy fermion compounds, which predicts an abrupt change in the size of the Fermi momentum.

  17. Electrostatic control over polarized currents through the spin-orbital Kondo effect

    NASA Astrophysics Data System (ADS)

    Büsser, C. A.; Feiguin, A. E.; Martins, G. B.

    2012-06-01

    Numerical calculations indicate that by suitably controlling the individual gate voltages of a capacitively coupled parallel double quantum dot, with each quantum dot coupled to one of two independent nonmagnetic channels, this system can be set into a spin-orbital Kondo state by applying a magnetic field. This Kondo regime, closely related to the SU(4) Kondo, flips spin from 1 to 0 through cotunneling processes that generate almost totally spin-polarized currents with opposite spin orientation along the two channels. Moreover, by appropriately changing the gate voltages of both quantum dots, one can simultaneously flip the spin polarization of the currents in each channel. As a similar zero magnetic field Kondo effect has been recently observed by Okazaki [Phys. Rev. BPLRBAQ1098-012110.1103/PhysRevB.84.161305 84, 161305(R) (2011)], we analyze a range of magnetic field values where this polarization effect seems robust, suggesting that the setup may be used as an efficient bipolar spin filter, which can generate electrostatically reversible spatially separated spin currents with opposite polarizations.

  18. Kondo effect in coupled quantum dots: a Non-crossing approximation study

    NASA Astrophysics Data System (ADS)

    Aguado, Ramon; Langreth, David

    2003-03-01

    The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson Hamiltonian with inter-impurity hopping. The Hamiltonian, formulated in slave-boson language, is solved by means of a generalization of the non-crossing approximation (NCA) to the present problem. We provide benchmark calculations of the predictions of the NCA for the linear and nonlinear transport properties of coupled quantum dots in the Kondo regime. We give a series of predictions that can be observed experimentally in linear and nonlinear transport measurements through coupled quantum dots. Importantly, it is demonstrated that measurements of the differential conductance G=dI/dV, for the appropriate values of voltages and inter-dot tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. This coherence can be also detected in the linear transport through the system: the curve linear conductance vs temperature is non-monotonic, with a maximum at a temperature T characterizing quantum coherence between both Kondo states.

  19. Environment-modulated Kondo phenomena in FePc/Au(111) adsorption systems

    NASA Astrophysics Data System (ADS)

    Wang, Yu; Zheng, Xiao; Yang, Jinlong

    2016-03-01

    Recent scanning tunneling microscopy experiments on electron transport through iron(II) phthalocyanine (FePc) molecules adsorbed on the Au(111) surface have revealed that the measured Kondo conductance signature depends strongly on the specific adsorption site. To understand the physical origin of experimental observations, particularly the variation of Kondo features with the molecular adsorption site, we employ a combined density functional theory (DFT) and hierarchical equations of motion (HEOM) approach to investigate the electronic structure and Kondo correlation in FePc/Au(111) composite systems. The calculation results indicate that, for the on-top adsorption configuration, the two degenerate spin-unpaired dπ orbitals on the Fe center are coupled indirectly through substrate band states, leading to the Fano-like antiresonance line shape in the d I /d V spectra, while for the bridge adsorption configuration, the environment-induced couplings are largely suppressed because of the two different spin-unpaired d orbitals. Therefore, our work suggests that the environment-induced coupling as an essential physical factor could greatly influence the Fano-Kondo features in magnetic molecule/metal composites, and the crucial role of local orbital degeneracy and symmetry is discovered. These findings provide important insights into the electron correlation effects in complex solid-state systems. The usefulness and practicality of the combined DFT+HEOM method is also highlighted.

  20. Conduction electron spin resonance in the α-Yb1-xFexAlB4 (0 ⩽ x ⩽ 0.50) and α-LuAlB4 compounds

    NASA Astrophysics Data System (ADS)

    Holanda, L. M.; Lesseux, G. G.; Magnavita, E. T.; Ribeiro, R. A.; Nakatsuji, S.; Kuga, K.; Fisk, Z.; Oseroff, S. B.; Urbano, R. R.; Rettori, C.; Pagliuso, P. G.

    2015-06-01

    β-YbAlB4 has become one of the most studied heavy fermion systems since its discovery due to its remarkable physical properties. This system is the first reported Yb-based heavy-fermion superconductor (HFS) for which the low-T superconducting state emerges from a non-fermi-liquid (NFL) normal state associated with quantum criticality Nakatsuji et al 2008 Nature 4 603. Additionally, it presents a striking and unprecedented electron spin resonance (ESR) signal which behaves as a conduction electron spin resonance (CESR) at high temperatures and acquires features of the Yb3+ local moment ESR at low temperatures. The latter, also named Kondo quasiparticles spin resonance (KQSR), has been defined as a 4f-ce strongly coupled ESR mode that behaves as a local probe of the Kondo quasiparticles in a quantum critical regime, Holanda et al 2011 Phys. Rev. Lett. 107 026402. Interestingly, β-YbAlB4 possesses a previously known structural variant, namely the α-YbAlB4, phase which is a paramagnetic Fermi liquid (FL) at low temperatures Macaluso et al 2007 Chem. Mater. 19 1918. However, it has been recently suggested that the α-YbAlB4 phase may be tuned to NFL behavior and/or magnetic ordering as the compound is doped with Fe. Here we report ESR studies on the α-Yb1-xFexAlB4 (0 ⩽ x ⩽ 0.50) series as well as on the reference compound α-LuAlB4. For all measured samples, the observed ESR signal behaves as a CESR in the entire temperature range (10 K ≲ T ≲ 300 K) in clear contrast with what has been observed for β-YbAlB4. This striking result indicates that the proximity to a quantum critical point is crucial to the occurrence of a KQSR signal.

  1. Using Combined X-ray Computed Tomography and Acoustic Resonance to Understand Supercritical CO2 Behavior in Fractured Sandstone

    NASA Astrophysics Data System (ADS)

    Kneafsey, T. J.; Nakagawa, S.

    2015-12-01

    Distribution of supercritical (sc) CO2 has a large impact on its flow behavior as well as on the properties of seismic waves used for monitoring. Simultaneous imaging of scCO2 distribution in a rock core using X-ray computed tomography (CT) and measurements of seismic waves in the laboratory can help understand how the distribution evolves as scCO2 invades through rock, and the resulting seismic signatures. To this end, we performed a series of laboratory scCO2 core-flood experiments in intact and fractured anisotropic Carbon Tan sandstone samples. In these experiments, we monitored changes in the CO2 saturation distribution and sonic-frequency acoustic resonances (yielding both seismic velocity and attenuation) over the course of the floods. A short-core resonant bar test system (Split-Hopkinson Resonant Bar Apparatus) custom fit into a long X-ray transparent pressure vessel was used for the seismic measurements, and a modified General Electric medical CT scanner was used to acquire X-ray CT data from which scCO2 saturation distributions were determined. The focus of the experiments was on the impact of single fractures on the scCO2 distribution and the seismic properties. For this reason, we examined several cases including 1. intact, 2. a closely mated fracture along the core axis, 3. a sheared fracture along the core axis (both vertical and horizontal for examining the buoyancy effect), and 4. a sheared fracture perpendicular to the core axis. For the intact and closely mated fractured cores, Young's modulus declined with increasing CO2 saturation, and attenuation increased up to about 15% CO2 saturation after which attenuation declined. For cores having wide axial fractures, the Young's modulus was lower than for the intact and closely mated cases, however did not change much with CO2 pore saturation. Much lower CO2 pore saturations were achieved in these cases. Attenuation increased more rapidly however than for the intact sample. For the core

  2. Kondo effects in a triangular triple quantum dot with lower symmetries

    NASA Astrophysics Data System (ADS)

    Oguri, A.; Amaha, S.; Nishikawa, Y.; Numata, T.; Shimamoto, M.; Hewson, A. C.; Tarucha, S.

    2011-05-01

    We study the low-energy properties and characteristic Kondo energy scale of a triangular triple quantum dot, connected to two non-interacting leads, in a wide parameter range of a gate voltage and distortions which lower the symmetry of an equilateral structure, using the numerical renormalization group approach. For large Coulomb interactions, the ground states with different characters can be classified according to the plateaus of Θ≡(δe-δo)(2/π), where δe and δo are the phase shifts for the even and odd partial waves. At these plateaus of Θ, both Θ and the occupation number Ntot≡(δe+δo)(2/π) take values close to integers, and thus the ground states can be characterized by these two integers. The Kondo effect with a local moment with total spin S=1 due to a Nagaoka mechanism appears on the plateau, which can be identified by Θ≃2.0 and Ntot≃4.0. For large distortions, however, the high-spin moment disappears through a singlet-triplet transition occurring within the four-electron region. It happens at a crossover to the adjacent plateaus for Θ≃0.0 and Θ≃4.0, and the two-terminal conductance has a peak in the transient regions. For weak distortions, the SU(4) Kondo effect also takes place for Ntot≃3.0. It appears as a sharp conductance valley between the S=1/2 Kondo ridges on both sides. We also find that the characteristic energy scale T* reflect these varieties of the Kondo effect. Particularly, T* is sensitive to the distribution of the charge and spin in the triangular triple dot.

  3. Stochastic resonance

    NASA Astrophysics Data System (ADS)

    Gammaitoni, Luca; Hänggi, Peter; Jung, Peter; Marchesoni, Fabio

    1998-01-01

    Over the last two decades, stochastic resonance has continuously attracted considerable attention. The term is given to a phenomenon that is manifest in nonlinear systems whereby generally feeble input information (such as a weak signal) can be be amplified and optimized by the assistance of noise. The effect requires three basic ingredients: (i) an energetic activation barrier or, more generally, a form of threshold; (ii) a weak coherent input (such as a periodic signal); (iii) a source of noise that is inherent in the system, or that adds to the coherent input. Given these features, the response of the system undergoes resonance-like behavior as a function of the noise level; hence the name stochastic resonance. The underlying mechanism is fairly simple and robust. As a consequence, stochastic resonance has been observed in a large variety of systems, including bistable ring lasers, semiconductor devices, chemical reactions, and mechanoreceptor cells in the tail fan of a crayfish. In this paper, the authors report, interpret, and extend much of the current understanding of the theory and physics of stochastic resonance. They introduce the readers to the basic features of stochastic resonance and its recent history. Definitions of the characteristic quantities that are important to quantify stochastic resonance, together with the most important tools necessary to actually compute those quantities, are presented. The essence of classical stochastic resonance theory is presented, and important applications of stochastic resonance in nonlinear optics, solid state devices, and neurophysiology are described and put into context with stochastic resonance theory. More elaborate and recent developments of stochastic resonance theory are discussed, ranging from fundamental quantum properties-being important at low temperatures-over spatiotemporal aspects in spatially distributed systems, to realizations in chaotic maps. In conclusion the authors summarize the achievements

  4. Direct observation of the spin texture in SmB6 as evidence of the topological Kondo insulator.

    PubMed

    Xu, N; Biswas, P K; Dil, J H; Dhaka, R S; Landolt, G; Muff, S; Matt, C E; Shi, X; Plumb, N C; Radović, M; Pomjakushina, E; Conder, K; Amato, A; Borisenko, S V; Yu, R; Weng, H-M; Fang, Z; Dai, X; Mesot, J; Ding, H; Shi, M

    2014-07-30

    Topological Kondo insulators have been proposed as a new class of topological insulators in which non-trivial surface states reside in the bulk Kondo band gap at low temperature due to strong spin-orbit coupling. In contrast to other three-dimensional topological insulators, a topological Kondo insulator is truly bulk insulating. Furthermore, strong electron correlations are present in the system, which may interact with the novel topological phase. By applying spin- and angle-resolved photoemission spectroscopy, here we show that the surface states of SmB6 are spin polarized. The spin is locked to the crystal momentum, fulfilling time reversal and crystal symmetries. Our results provide strong evidence that SmB6 can host topological surface states in a bulk insulating gap stemming from the Kondo effect, which can serve as an ideal platform for investigating of the interplay between novel topological quantum states with emergent effects and competing orders induced by strongly correlated electrons.

  5. Cyclotron dynamics of a Kondo singlet in a spin-orbit-coupled alkaline-earth-metal atomic gas

    NASA Astrophysics Data System (ADS)

    Jiang, Bo-Nan; Lv, Hao; Wang, Wen-Li; Du, Juan; Qian, Jun; Wang, Yu-Zhu

    2014-11-01

    We propose a scheme to investigate the interplay between the Kondo-exchange interaction and the quantum spin Hall effect with ultracold fermionic alkaline-earth-metal atoms trapped in two-dimensional optical lattices using ultracold collision and laser-assisted tunneling. In the strong Kondo-coupling regime, although the loop trajectory of the mobile atom disappears, collective dynamics of an atom pair in two clock states can exhibit an unexpected spin-dependent cyclotron orbit in a plaquette, realizing the quantum spin Hall effect of the Kondo singlet. We demonstrate that the collective cyclotron dynamics of the spin-zero Kondo singlet is governed by an effective Harper-Hofstadter model in addition to second-order diagonal tunneling.

  6. Genome sequence of Frateuria aurantia type strain (Kondo 67(T)), a xanthomonade isolated from Lilium auratium Lindl.

    SciTech Connect

    Anderson, Iain; Teshima, Hazuki; Nolan, Matt; Lapidus, Alla L.; Tice, Hope; Glavina Del Rio, Tijana; Cheng, Jan-Fang; Han, Cliff; Tapia, Roxanne; Goodwin, Lynne A.; Pitluck, Sam; Liolios, Konstantinos; Mavromatis, K; Pagani, Ioanna; Ivanova, N; Mikhailova, Natalia; Pati, Amrita; Chen, Amy; Palaniappan, Krishna; Land, Miriam L; Rohde, Manfred; Lang, Elke; Detter, J. Chris; Goker, Markus; Woyke, Tanja; Bristow, James; Eisen, Jonathan; Markowitz, Victor; Hugenholtz, Philip; Kyrpides, Nikos C; Klenk, Hans-Peter

    2013-01-01

    rateuria aurantia (ex Kondo and Ameyama 1958) Swings et al. 1980 is a member of the bispecific genus Frateuria in the family Xanthomonadaceae, which is already heavily targeted for non-type strain genome sequencing. Strain Kondo 67(T) was initially (1958) identified as a member of 'Acetobacter aurantius', a name that was not considered for the approved list. Kondo 67(T) was therefore later designated as the type strain of the newly proposed acetogenic species Frateuria aurantia. The strain is of interest because of its triterpenoids (hopane family). F. aurantia Kondo 67(T) is the first member of the genus Frateura whose genome sequence has been deciphered, and here we describe the features of this organism, together with the complete genome sequence and annotation. The 3,603,458-bp long chromosome with its 3,200 protein-coding and 88 RNA genes is a part of the Genomic Encyclopedia of Bacteria and Archaea project.

  7. Surface Plasmon Resonance Fiber Sensor for Real-Time and Label-Free Monitoring of Cellular Behavior

    PubMed Central

    Shevchenko, Yanina; Camci-Unal, Gulden; Cuttica, Davide F.; Dokmeci, Mehmet R.; Albert, Jacques; Khademhosseini, Ali

    2014-01-01

    This paper reports on the application of an optical fiber biosensor for real-time analysis of cellular behavior. Our findings illustrate that a fiber sensor manufactured from a traditional telecommunication fiber can be integrated into conventional cell culture equipment and used for real-time and label-free monitoring of cellular responses to chemical stimuli. The sensing mechanism used for the measurement of cellular responses is based on the excitation of Surface Plasmon Resonance (SPR) on the surface of the optical fiber. In this proof of concept study, the sensor was utilized to investigate the influence of a number of different stimuli on cells - we tested the effects of trypsin, serum and sodium azide. These stimuli induced detachment of cells from the sensor surface, uptake of serum and inhibition of cellular metabolism, accordingly. The effects of different stimuli were confirmed with alamar blue assay, phase contrast and fluorescence microscopy. The results indicated that the fiber biosensor can be successfully utilized for real-time and label-free monitoring of cellular response in the first 30 minutes following the introduction of a stimulus. Furthermore, we demonstrated that the optical fiber biosensors can be easily regenerated for repeated use, proving this platform as a versatile and cost-effective sensing tool. PMID:24549115

  8. Free radical scavenging activities measured by electron spin resonance spectroscopy and B16 cell antiproliferative behaviors of seven plants.

    PubMed

    Calliste, C A; Trouillas, P; Allais, D P; Simon, A; Duroux, J L

    2001-07-01

    In an effort to discover new antioxidant natural compounds, seven plants that grow in France (most of them in the Limousin countryside) were screened. Among these plants, was the extensively studied Vitis vinifera as reference. For each plant, sequential percolation was realized with five solvents of increasing polarities (hexane, chloroform, ethyl acetate, methanol, and water). Free radical scavenging activities were examined in different systems using electron spin resonance (ESR) spectroscopy. These assays were based on the stable free radical 1,1-diphenyl-2-picrylhydrazyl (DPPH), the hydroxyl radicals generated by a Fenton reaction, and the superoxide radicals generated by the X/XO system. Antiproliferative behavior was studied on B16 melanoma cells. ESR results showed that three plants (Castanea sativa, Filipendula ulmaria, and Betula pendula) possessed, for the most polar fractions (presence of phenolic compounds), high antioxidant activities in comparison with the Vitis vinifera reference. Gentiana lutea was the only one that presented a hydroxyl scavenging activity for the ethyl acetate and chloroform fractions. The antiproliferative test results showed that the same three plants are the most effective, but for the apolar fractions (chloroform and hexane).

  9. Introducing the Hyper Hadrons, Hyper Mesons, Heavy Leptons and Massive Neutrinos of Kazuo Kondo's Mass Quantum Cascade

    NASA Astrophysics Data System (ADS)

    Croll, Grenville J.

    The late Professor Kazuo Kondo (Department of Mathematics, Tokyo University, Japan) l a hitherto unknown a priori particle theory which provides predictions of massive particles which may be detected by the Large Hadron Collider (LHC) and related apparatus. This article briefly introduces Kondo's work and documents the derivation and masses of his expected hyper-mesons, hyper-hadrons, heavy leptons and massive neutrinos. Several particles in these classes may have already been detected.

  10. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2-δAs2.

    PubMed

    Luo, Yongkang; Ronning, F; Wakeham, N; Lu, Xin; Park, Tuson; Xu, Z-A; Thompson, J D

    2015-11-01

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2-δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 E-/formular unit in CeNi2-δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. The small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening. PMID:26483465

  11. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2−δAs2

    PubMed Central

    Luo, Yongkang; Ronning, F.; Wakeham, N.; Lu, Xin; Park, Tuson; Xu, Z.-A.; Thompson, J. D.

    2015-01-01

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2−δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ∼0.032 e−/formular unit in CeNi2−δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. The small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening. PMID:26483465

  12. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2–δAs2

    DOE PAGES

    Luo, Yongkang; Ronning, F.; Wakeham, N.; Lu, Xin; Park, Tuson; Xu, Z. -A.; Thompson, J. D.

    2015-10-19

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2–δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressuremore » and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 e–/formular unit in CeNi2–δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. Here, the small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening.« less

  13. Influence of gamma radiation and magnetic resonance imaging radiation on micro-structure, hardness and electrochemical corrosion behavior of Co‒Cr-based dental alloy

    NASA Astrophysics Data System (ADS)

    Bakr El-Bediwi, Abu; Saada, Mohamed; El-Fallal, Abeer A.; El-Khaligy, Samar

    2011-03-01

    The effects of therapeutic gamma radiation at 10, 20 and 30 kGy and magnetic resonance imaging radiation from a 1.5 T MR scanner on the micro-structure, electrochemical corrosion behavior and micro-hardness of commercial dental Magnum H50 (Co=64%, Cr=29%, Mo=6.5%) alloy have been investigated. The corrosion rate, corrosion resistance, corrosion potential and corrosion current density values of the alloy treated with 0.5 M HCl vary due to gamma and magnetic resonance imaging radiation. At 30 kGy, the corrosion resistance of Magnum H50 reaches a minimum value and the corrosion rate obtains a maximum value. The Vickers hardness value of the Magnum H50 alloy decreases after both gamma and magnetic resonance imaging radiation.

  14. Incoherence-coherence crossover and low-temperature Fermi-liquid-like behavior in AFe2As2 (A  =  K, Rb, Cs): evidence from electrical transport properties.

    PubMed

    Xiang, Z J; Wang, N Z; Wang, A F; Zhao, D; Sun, Z L; Luo, X G; Wu, T; Chen, X H

    2016-10-26

    We study the normal-state transport properties of AFe2As2 (A  =  K, Rb and Cs) single crystals using Hall coefficient, resistivity and magnetoresistance (MR) measurements. In all three materials, the Hall coefficient R H shows a strong temperature dependence, which is typical for multi-band systems. In particular, R H develops an upturn below a characteristic temperature [Formula: see text], which is in agreement with the incoherence-coherence crossover reported in recent nuclear magnetic resonance studies. A Fermi-liquid-like state, characterized by T (2) behavior of the resistivity and a positive orbital MR obeying Kohler's rule, emerges below T FL  ∼0.4 [Formula: see text]. The superconducting transition temperature T c experiences a simultaneous suppression with [Formula: see text] and T FL as the alkali ion's radius increases from A  =  K to A  =  Cs, suggesting that the unconventional superconductivity in the AFe2As2 series is related to the strength of the electronic coherence. A phase diagram, similar to that in the heavy fermion Kondo lattice system, is obtained. Based on all the experimental evidence, we argue that the physical properties of this family of heavily hole-doped Fe-based superconductors are controlled by the hybridization between itinerant carriers and localized orbitals, and the Kondo scenario could be effective in such a case.

  15. Incoherence-coherence crossover and low-temperature Fermi-liquid-like behavior in AFe2As2 (A  =  K, Rb, Cs): evidence from electrical transport properties

    NASA Astrophysics Data System (ADS)

    Xiang, Z. J.; Wang, N. Z.; Wang, A. F.; Zhao, D.; Sun, Z. L.; Luo, X. G.; Wu, T.; Chen, X. H.

    2016-10-01

    We study the normal-state transport properties of AFe2As2 (A  =  K, Rb and Cs) single crystals using Hall coefficient, resistivity and magnetoresistance (MR) measurements. In all three materials, the Hall coefficient R H shows a strong temperature dependence, which is typical for multi-band systems. In particular, R H develops an upturn below a characteristic temperature {{T}\\ast} , which is in agreement with the incoherence-coherence crossover reported in recent nuclear magnetic resonance studies. A Fermi-liquid-like state, characterized by T 2 behavior of the resistivity and a positive orbital MR obeying Kohler’s rule, emerges below T FL  ˜0.4 ~{{T}\\ast} . The superconducting transition temperature T c experiences a simultaneous suppression with {{T}\\ast} and T FL as the alkali ion’s radius increases from A  =  K to A  =  Cs, suggesting that the unconventional superconductivity in the AFe2As2 series is related to the strength of the electronic coherence. A phase diagram, similar to that in the heavy fermion Kondo lattice system, is obtained. Based on all the experimental evidence, we argue that the physical properties of this family of heavily hole-doped Fe-based superconductors are controlled by the hybridization between itinerant carriers and localized orbitals, and the Kondo scenario could be effective in such a case.

  16. Incoherence-coherence crossover and low-temperature Fermi-liquid-like behavior in AFe2As2 (A  =  K, Rb, Cs): evidence from electrical transport properties.

    PubMed

    Xiang, Z J; Wang, N Z; Wang, A F; Zhao, D; Sun, Z L; Luo, X G; Wu, T; Chen, X H

    2016-10-26

    We study the normal-state transport properties of AFe2As2 (A  =  K, Rb and Cs) single crystals using Hall coefficient, resistivity and magnetoresistance (MR) measurements. In all three materials, the Hall coefficient R H shows a strong temperature dependence, which is typical for multi-band systems. In particular, R H develops an upturn below a characteristic temperature [Formula: see text], which is in agreement with the incoherence-coherence crossover reported in recent nuclear magnetic resonance studies. A Fermi-liquid-like state, characterized by T (2) behavior of the resistivity and a positive orbital MR obeying Kohler's rule, emerges below T FL  ∼0.4 [Formula: see text]. The superconducting transition temperature T c experiences a simultaneous suppression with [Formula: see text] and T FL as the alkali ion's radius increases from A  =  K to A  =  Cs, suggesting that the unconventional superconductivity in the AFe2As2 series is related to the strength of the electronic coherence. A phase diagram, similar to that in the heavy fermion Kondo lattice system, is obtained. Based on all the experimental evidence, we argue that the physical properties of this family of heavily hole-doped Fe-based superconductors are controlled by the hybridization between itinerant carriers and localized orbitals, and the Kondo scenario could be effective in such a case. PMID:27589485

  17. Gate-tunable Kondo resistivity and dephasing rate in graphene studied by numerical renormalization group calculations

    NASA Astrophysics Data System (ADS)

    Lo, Po-Wei; Guo, Guang-Yu; Anders, Frithjof B.

    2014-05-01

    Motivated by the recent observation of the Kondo effect in graphene in transport experiments, we investigate the resistivity and dephasing rate in the Kondo regime due to magnetic impurities in graphene with different chemical potentials (μ). The Kondo effect due to either carbon vacancies or magnetic adatoms in graphene is described by the single-orbital pseudogap asymmetric Anderson impurity model which is solved by the accurate numerical renormalization group method. We find that although the Anderson impurity model considered here is a mixed-valence system, it can be driven into either the Kondo [μ >μc (critical value) >0], mixed-valency (μ ≈μc), or empty-orbital (μ <μc) regime by a gate voltage, giving rise to characteristic features in resistivity and dephasing rate in each regime. Specifically, in the case of μ <μc, the shapes of the resistivity (dephasing rate) curves for different μ are nearly identical. However, as temperature decreases, they start to increase to their maxima at a lower T /TK, but more rapidly [as (TK/T)3/2] than in normal metals [here, T (TK) denotes the (Kondo) temperature]. As T further decreases, after reaching the maximum, the dephasing rate drops more quickly than in normal metals, behaving as (T/TK)3 instead of (T/TK)2. Furthermore, the resistivity has a distinct peak above the saturation value near TK. In the case of μ >μc, in contrast, the resistivity curve has an additional broad shoulder above 10TK and the dephasing rate exhibits an interesting shoulder-peak shape. In the narrow boundary region (μ ≈μc), both the resistivity and dephasing rate curves are similar to the corresponding ones in normal metals. This explains the conventional Kondo-like resistivity from recent experiments on graphene with defects, although the distinct features in the resistivity in the other cases (μ <μc or μ >μc) were not seen in the experiments. The interesting features in the resistivity and dephasing rate are analyzed in

  18. Models for Copper Dynamic Behavior in Doped Cadmium dl-Histidine Crystals: Electron Paramagnetic Resonance and Crystallographic Analysis.

    PubMed

    Colaneri, Michael J; Teat, Simon J; Vitali, Jacqueline

    2015-11-12

    Electron paramagnetic resonance and crystallographic studies of copper-doped cadmium dl-histidine, abbreviated as CdDLHis, were undertaken to gain further understanding on the relationship between site structure and dynamic behavior in biological model complexes. X-ray diffraction measurements determined the crystal structure of CdDLHis at 100 and 298 K. CdDLHis crystallizes in the monoclinic space group P21/c with two cadmium complexes per asymmetric unit. In each complex, the Cd is hexacoordinated to two histidine molecules. Both histidines are l in one complex and d in the other. Additionally, each complex contains multiple waters of varying disorder. Single crystal EPR spectroscopic splitting (g) and copper hyperfine (A(Cu)) tensors at room temperature (principal values: g = 2.249, 2.089, 2.050; A(Cu) = -453, -30.5, -0.08 MHz) were determined from rotational experiments. Alignments of the tensor directions with the host structure were used to position the copper unpaired dx(2)-y(2) orbital in an approximate plane made by four proposed ligand atoms: the N-imidazole and N-amino of one histidine, and the N-amino and O-carboxyl of the other. Each complex has two such planes related by noncrystallographic symmetry, which make an angle of 65° and have a 1.56 Å distance between their midpoints. These findings are consistent with three interpretations that can adequately explain previous temperature-dependent EPR powder spectra of this system: (1) a local structural distortion (static strain) at the copper site has a temperature dependence significant enough to affect the EPR pattern, (2) the copper can hop between the two sites in each complex at high temperature, and (3) there exists a dynamic Jahn-Teller effect involving the copper ligands. PMID:26501364

  19. Superconductivity of composite particles in a two-channel Kondo lattice.

    PubMed

    Hoshino, Shintaro; Kuramoto, Yoshio

    2014-04-25

    Emergence of odd-frequency s-wave superconductivity is demonstrated in the two-channel Kondo lattice by means of the dynamical mean-field theory combined with the continuous-time quantum Monte Carlo method. Around half filling of the conduction bands, divergence of an odd-frequency pairing susceptibility is found, which signals instability toward the superconductivity. The corresponding order parameter is equivalent to a staggered composite-pair amplitude with even frequencies, which involves both localized spins and conduction electrons. A model wave function is constructed for the composite order with the use of symmetry operations such as charge conjugation and channel rotations. Given a certain asymmetry of the conduction bands, another s-wave superconductivity is found that has a uniform order parameter. The Kondo effect in the presence of two channels is essential for both types of unconventional superconductivity.

  20. Quantum critical Mott transitions in a bilayer Kondo insulator-metal model system

    NASA Astrophysics Data System (ADS)

    Sen, Sudeshna; Vidhyadhiraja, N. S.

    2016-04-01

    A bilayer system comprising a Kondo insulator coupled to a simple metal (KI-M) is considered. Employing the framework of dynamical mean-field theory, the model system is shown to exhibit a surface of quantum critical points (QCPs) that separates a Kondo screened, Fermi liquid phase from a local moment, Mott insulating phase. The quantum critical nature of these Mott transitions is characterized by the vanishing of (a) the coherence scale on the Fermi liquid side, and (b) the Mott gap on the MI side. In contrast to the usual "large-to-small" Fermi surface (FS) QCPs in heavy-fermion systems, the bilayer KI-M system exhibits a complete FS destruction.

  1. Nonequilibrium transport through a Kondo dot in a magnetic field: perturbation theory and poor man's scaling.

    PubMed

    Rosch, A; Paaske, J; Kroha, J; Wölfle, P

    2003-02-21

    We consider electron transport through a quantum dot described by the Kondo model in the regime of large transport voltage V in the presence of a magnetic field B with max((V,B)>T(K). The electric current I and the local magnetization M are found to be universal functions of V/T(K) and B/T(K), where T(K) is the equilibrium Kondo temperature. We present a generalization of the perturbative renormali-zation group to frequency dependent coupling functions, as necessitated by the structure of bare perturbation theory. We calculate I and M within a poor man's scaling approach and find excellent agreement with experiment. PMID:12633260

  2. Kondo lattice on the edge of a 2D topological insulator

    NASA Astrophysics Data System (ADS)

    Maciejko, Joseph

    2012-02-01

    Much attention has been devoted recently to the experimental and theoretical study of the effect of magnetic impurities on the stability of the gapless boundary modes of topological insulators. When the quantum dynamics of the impurities is considered, those boundary modes constitute novel types of fermionic baths which may affect the nature of possible impurity phases and phase transitions. We study a regular one-dimensional array of quantum magnetic impurities interacting with the helical edge liquid of a two-dimensional time-reversal invariant topological insulator. Exact solutions at the special Toulouse and Luther-Emery points as well as a renormalization group analysis àla Anderson-Yuval allow us to construct a phase diagram in the space of Kondo coupling, electron-electron interaction strength, and electron density. We point out similarities and differences with the Kondo lattice in a ordinary one-dimensional electron gas.

  3. Evidence for charge Kondo effect in superconducting Tl-doped PbTe

    SciTech Connect

    Fisher, I

    2010-01-11

    We report results of low-temperature thermodynamic and transport measurements of Pb{sub 1-x}Tl{sub x}Te single crystals for Tl concentrations up to the solubility limit of approximately x = 1.5%. For all doped samples, we observe a low-temperature resistivity upturn that scales in magnitude with the Tl concentration. The temperature and field dependence of this upturn are consistent with a charge Kondo effect involving degenerate Tl valence states differing by two electrons, with a characteristic Kondo temperature T{sub K} {approx} 6 K. The observation of such an effect supports an electronic pairing mechanism for superconductivity in this material and may account for the anomalously high T{sub c} values.

  4. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    PubMed Central

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; Gu, Genda; Mason, Nadya

    2016-01-01

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. We characterize the zero-bias peaks and discuss their origin. PMID:26911258

  5. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    DOE PAGES

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; Gu, Genda; Mason, Nadya

    2016-02-25

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. As a result, we characterize the zero-bias peaks and discuss their origin.

  6. Emergence of anisotropic heavy fermions in antiferromagnetic Kondo lattice CeIn3 revealed by photoemission

    NASA Astrophysics Data System (ADS)

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Zhang, Wen; Lai, Xinchun; Donglai Feng Team; Huiqiu Yuan Team

    One basic concept in heavy fermions systems is the entanglement of localized spin state and itinerant electron state. It can be tuned by two competitive intrinsic mechanisms, Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction, with external disturbances. The key issue regarding heavy fermions properties is how the two mechanisms work in the same phase region. To investigate the relation of the two mechanisms, the cubic antiferromagnetic heavy fermions compound CeIn3 was investigated by soft x-ray angle resolved photoemission spectroscopy. The hybridization between f electrons and conduction bands in the paramagnetic state was observed directly, providing compelling evidence for Kondo screening scenario and coexistence of two mechanisms. The hybridization strength shows slight and regular anisotropy in K space, implying that the two mechanisms are competitive and anisotropic. This work illuminates the concomitant and competitive relation between the two mechanisms and supplies some evidences for the anisotropic superconductivity of CeIn3

  7. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire

    NASA Astrophysics Data System (ADS)

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A.; Gu, Genda; Mason, Nadya

    2016-02-01

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires—for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi1.33Sb0.67)Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. We characterize the zero-bias peaks and discuss their origin.

  8. Kondo-like zero-bias conductance anomaly in a three-dimensional topological insulator nanowire.

    PubMed

    Cho, Sungjae; Zhong, Ruidan; Schneeloch, John A; Gu, Genda; Mason, Nadya

    2016-02-25

    Zero-bias anomalies in topological nanowires have recently captured significant attention, as they are possible signatures of Majorana modes. Yet there are many other possible origins of zero-bias peaks in nanowires--for example, weak localization, Andreev bound states, or the Kondo effect. Here, we discuss observations of differential-conductance peaks at zero-bias voltage in non-superconducting electronic transport through a 3D topological insulator (Bi(1.33)Sb(0.67))Se3 nanowire. The zero-bias conductance peaks show logarithmic temperature dependence and often linear splitting with magnetic fields, both of which are signatures of the Kondo effect in quantum dots. We characterize the zero-bias peaks and discuss their origin.

  9. Competition between Kondo and RKKY correlations in the presence of strong randomness.

    PubMed

    Tran, Minh-Tien; Kim, Ki-Seok

    2011-10-26

    We propose that competition between Kondo and magnetic correlations results in a novel universality class for heavy fermion quantum criticality in the presence of strong randomness. Starting from an Anderson lattice model with disorder, we derive an effective local field theory in the dynamical mean-field theory approximation, where randomness is introduced into both hybridization and Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions. Performing the saddle-point analysis in the U(1) slave-boson representation, we reveal its phase diagram which shows a quantum phase transition from a spin liquid state to a local Fermi liquid phase. In contrast with the clean limit case of the Anderson lattice model, the effective hybridization given by holon condensation turns out to vanish, resulting from the zero mean value of the hybridization coupling constant. However, we show that the holon density becomes finite when the variance of the hybridization is sufficiently larger than that of the RKKY coupling, giving rise to the Kondo effect. On the other hand, when the variance of the hybridization becomes smaller than that of the RKKY coupling, the Kondo effect disappears, resulting in a fully symmetric paramagnetic state, adiabatically connected to the spin liquid state of the disordered Heisenberg model. We investigate the quantum critical point beyond the mean-field approximation. Introducing quantum corrections fully self-consistently in the non-crossing approximation, we prove that the local charge susceptibility has exactly the same critical exponent as the local spin susceptibility, suggesting an enhanced symmetry at the local quantum critical point. This leads us to propose novel duality between the Kondo singlet phase and the critical local moment state beyond the Landau-Ginzburg-Wilson paradigm. The Landau-Ginzburg-Wilson forbidden duality serves the mechanism of electron fractionalization in critical impurity dynamics, where such fractionalized excitations are

  10. Kondo spin screening cloud in two-dimensional electron gas with spin-orbit couplings.

    PubMed

    Feng, Xiao-Yong; Zhang, Fu-Chun

    2011-03-16

    A spin-1/2 Anderson impurity in a semiconductor quantum well with Rashba and Dresselhaus spin-orbit couplings is studied by using a variational wavefunction method. The local magnetic moment is found to be quenched at low temperatures. The spin-spin correlations of the impurity and the conduction electron density show anisotropy in both spatial and spin spaces, which interpolates the Kondo spin screenings of a conventional metal and of a surface of three-dimensional topological insulators.

  11. Localization at the edge of a 2D topological insulator by Kondo impurities with random anisotropies.

    PubMed

    Altshuler, B L; Aleiner, I L; Yudson, V I

    2013-08-23

    We consider chiral electrons moving along the one-dimensional helical edge of a two-dimensional topological insulator and interacting with a disordered chain of Kondo impurities. Assuming the electron-spin couplings of random anisotropies, we map this system to the problem of the pinning of the charge density wave by the disordered potential. This mapping proves that arbitrary weak anisotropic disorder in coupling of chiral electrons with spin impurities leads to the Anderson localization of the edge states.

  12. Spin fluctuations in the anisotropic Kondo insulator CeRu4 Sn6

    NASA Astrophysics Data System (ADS)

    Fuhrman, Wesley T.; Haenel, J.; Rodriguez, J.; Paschen, S.; Broholm, C. L.

    We report and model anisotropic quasi-elastic magnetic neutron scattering from single crystalline CeRu4Sn6. For T ~ 2 K the magnetic neutron scattering is broad in momentum (Q) with a persistent 1 / ℏω spectrum throughout the Brillouin zone. This indicates a lack of spatial coherence and no characteristic energy scale beyond the 0.2 meV resolution of the measurement. We find the Q-dependence of the scattering can be modeled by a Kondo-Heisenberg Hamiltonian that describes residual carriers and incompletely compensated localized electrons. These findings support the interpretation of tetragonal CeRu4Sn6 as an anisotropic or nodal Kondo insulator, markedly different from typical cubic Kondo insulators. We further discuss potential topological implications. Work at IQM was supported by the U.S. Department of Energy, office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-08ER4654. W.T.F. thanks the ARCS foundation and Lockheed Martin for additional support.

  13. Transport in a hybrid normal metal/topological superconductor Kondo model

    NASA Astrophysics Data System (ADS)

    Chirla, Razvan; Dinu, I. V.; Moldoveanu, V.; Moca, Cǎtǎlin Paşcu

    2014-11-01

    We investigate the equilibrium and nonequilibrium transport through a quantum dot in the Kondo regime, embedded between a normal metal and a topological superconductor supporting Majorana bound states at its end points. We find that the Kondo physics is significantly modified by the presence of the Majorana modes. When the Majorana modes are coupled, aside from the Kondo scale TK, a new energy scale T*≪TK emerges, that controls the low-energy physics of the system. At low temperatures, the ac conductance is suppressed for frequencies below T*, while the noise spectrum acquires a ˜ω3 dependence. At high temperatures, T ≫TK , the regular logarithmic dependence in the differential conductance is also affected. Under nonequilibrium conditions, and in particular in the {T ,B }→0 limit, the differential conductance becomes negative. These findings indicate that the changes in transport may serve as clues for detecting the Majorana bound states in such systems. In terms of methods used, we characterize the transport by using a combination of perturbative and renormalization-group approaches.

  14. Controlling Kondo-like Scattering at the SrTiO3-based Interfaces

    PubMed Central

    Han, K.; Palina, N.; Zeng, S. W.; Huang, Z.; Li, C. J.; Zhou, W. X.; Wan, D.-Y.; Zhang, L. C.; Chi, X.; Guo, R.; Chen, J. S.; Venkatesan, T.; Rusydi, A.; Ariando, A

    2016-01-01

    The observation of magnetic interaction at the interface between nonmagnetic oxides has attracted much attention in recent years. In this report, we show that the Kondo-like scattering at the SrTiO3-based conducting interface is enhanced by increasing the lattice mismatch and growth oxygen pressure PO2. For the 26-unit-cell LaAlO3/SrTiO3 (LAO/STO) interface with lattice mismatch being 3.0%, the Kondo-like scattering is observed when PO2 is beyond 1 mTorr. By contrast, when the lattice mismatch is reduced to 1.0% at the (La0.3Sr0.7)(Al0.65Ta0.35)O3/SrTiO3 (LSAT/STO) interface, the metallic state is always preserved up to PO2 of 100 mTorr. The data from Hall measurement and X-ray absorption near edge structure (XANES) spectroscopy reveal that the larger amount of localized Ti3+ ions are formed at the LAO/STO interface compared to LSAT/STO. Those localized Ti3+ ions with unpaired electrons can be spin-polarized to scatter mobile electrons, responsible for the Kondo-like scattering observed at the LAO/STO interface. PMID:27147407

  15. Controlling Kondo-like Scattering at the SrTiO3-based Interfaces.

    PubMed

    Han, K; Palina, N; Zeng, S W; Huang, Z; Li, C J; Zhou, W X; Wan, D-Y; Zhang, L C; Chi, X; Guo, R; Chen, J S; Venkatesan, T; Rusydi, A; Ariando

    2016-05-05

    The observation of magnetic interaction at the interface between nonmagnetic oxides has attracted much attention in recent years. In this report, we show that the Kondo-like scattering at the SrTiO3-based conducting interface is enhanced by increasing the lattice mismatch and growth oxygen pressure PO2. For the 26-unit-cell LaAlO3/SrTiO3 (LAO/STO) interface with lattice mismatch being 3.0%, the Kondo-like scattering is observed when PO2 is beyond 1 mTorr. By contrast, when the lattice mismatch is reduced to 1.0% at the (La0.3Sr0.7)(Al0.65Ta0.35)O3/SrTiO3 (LSAT/STO) interface, the metallic state is always preserved up to PO2 of 100 mTorr. The data from Hall measurement and X-ray absorption near edge structure (XANES) spectroscopy reveal that the larger amount of localized Ti(3+) ions are formed at the LAO/STO interface compared to LSAT/STO. Those localized Ti(3+) ions with unpaired electrons can be spin-polarized to scatter mobile electrons, responsible for the Kondo-like scattering observed at the LAO/STO interface.

  16. Theory of low energy excitations in resonant inelastic x-ray scattering for rare-earth systems: Yb compounds as typical examples

    NASA Astrophysics Data System (ADS)

    Kotani, A.

    2011-04-01

    Theoretical predictions are given for low energy excitations, such as crystal field excitations and Kondo resonance excitations, to be detected by high-resolution measurements of resonant inelastic x-ray scattering (RIXS) of rare-earth materials with Yb compounds as typical examples. Crystal field excitations in the Yb 3d RIXS of a Yb3+ ion in the cubic crystal field are formulated, and the calculation of RIXS spectra for YbN is done. Kondo resonance excitations revealed in the Yb 3d RIXS spectra are calculated for mixed-valence Yb compounds, Yb1-xLuxAl3, in the leading term approximation of the 1/Nf expansion method with a single impurity Anderson model. It is emphasized that the high-resolution RIXS with polarization dependence is a powerful tool to study the crystal field levels together with their symmetry and also the Kondo bound state in rare-earth compounds. Some in-depth discussions are given on the polarization effects of RIXS, including 4d and 2p RIXS spectra, the coherence effect of the Kondo bound states, and the importance of the high-resolution RIXS spectra for condensed matter physics under extreme conditions.

  17. PRESS echo time behavior of triglyceride resonances at 1.5 T: Detecting ω-3 fatty acids in adipose tissue in vivo

    NASA Astrophysics Data System (ADS)

    Lundbom, Jesper; Heikkinen, Sami; Fielding, Barbara; Hakkarainen, Antti; Taskinen, Marja-Riitta; Lundbom, Nina

    2009-11-01

    AimThis study investigated the impact of fatty acid (FA) composition on the echo time behavior of triglyceride resonances in a clinical setting. The feasibility of 1H NMR spectroscopy to detect these resonances was also evaluated in human adipose tissue in vivo. MethodTen edible oils chosen to cover a wide spectrum of FA compositions were used as phantom material. The detailed FA composition and intrinsic proton spectra of the oils were characterized by gas chromatography and high-resolution 1H NMR spectroscopy (11.7 T), respectively. The detailed echo time behavior of the oils were subsequently measured by 1H NMR spectroscopy in a clinical scanner (1.5 T) using PRESS. The effect of temperature was investigated in five oils. ResultsThe olefinic (5.3 ppm) and diallylic (2.8 ppm) resonances exhibited distinct J-modulation patterns independent of oil FA composition. The methylene resonance (1.3 ppm) displayed an exponential decay, with the apparent T2 showing a weak positive correlation with oil unsaturation ( R = 0.628, P = 0.052), probably a result of changes in viscosity. For the methyl resonance (0.9 ppm), oils high in ω-3 FA displayed a markedly different J-modulation pattern compared to non-ω-3 oils. The characteristic J-modulation of the ω-3 methyl group could be attributed to the phase behavior of the ω-3 methyl triplet signal (all triplet lines in-phase at TE of 135 ms), a result of the ω-3 methyl end forming a first order spin system. The ω-3 methyl outer triplet line at 1.08 ppm of the TE = 140 ms spectrum was found to be useful for determining the ω-3 content of the oils ( R = 0.999, standard error of estimate (SE) 0.80). The olefinic and diallylic proton resonance (measured at TE = 50 ms) areas correlated with the olefinic ( R = 0.993, SE 0.33) and diallylic ( R = 0.997, SE 0.19) proton contents calculated from the GC data. Information derived from long echo time spectra (TE = 200) demonstrated good correlations to GC data and showed no change with

  18. Long range order and two-fluid behavior in heavy electron materials

    DOE PAGES

    Shirer, Kent R.; Shockley, Abigail C.; Dioguardi, Adam P.; Crocker, John; Lin, Ching H.; apRoberts-Warren, Nicholas; Nisson, David M.; Klavins, Peter; Cooley, Jason C.; Yang, Yi -feng; et al

    2012-09-24

    The heavy electron Kondo liquid is an emergent state of condensed matter that displays universal behavior independent of material details. Properties of the heavy electron liquid are best probed by NMR Knight shift measurements, which provide a direct measure of the behavior of the heavy electron liquid that emerges below the Kondo lattice coherence temperature as the lattice of local moments hybridizes with the background conduction electrons. Because the transfer of spectral weight between the localized and itinerant electronic degrees of freedom is gradual, the Kondo liquid typically coexists with the local moment component until the material orders at lowmore » temperatures. The two-fluid formula captures this behavior in a broad range of materials in the paramagnetic state. In order to investigate two-fluid behavior and the onset and physical origin of different long range ordered ground states in heavy electron materials, we have extended Knight shift measurements to URu2Si2, CeIrIn5, and CeRhIn5. In CeRhIn5 we find that the antiferromagnetic order is preceded by a relocalization of the Kondo liquid, providing independent evidence for a local moment origin of antiferromagnetism. In URu2Si2 the hidden order is shown to emerge directly from the Kondo liquid and so is not associated with local moment physics. Lastly, our results imply that the nature of the ground state is strongly coupled with the hybridization in the Kondo lattice in agreement with phase diagram proposed by Yang and Pines.« less

  19. Field-Enhanced Kondo Correlations in a Half-Filling Nanotube Dot: Evolution of an SU(N) Fermi-Liquid Fixed Point

    NASA Astrophysics Data System (ADS)

    Teratani, Yoshimichi; Sakano, Rui; Fujiwara, Ryo; Hata, Tokuro; Arakawa, Tomonori; Ferrier, Meydi; Kobayashi, Kensuke; Oguri, Akira

    2016-09-01

    Carbon nanotube quantum dot has four-fold degenerate one-particle levels, which bring a variety to the Kondo effects taking place in a wide tunable-parameter space. We theoretically study an emergent SU(2) symmetry that is suggested by recent magneto-transport measurements, carried out near two electrons filling. It does not couple with the magnetic field, and emerges in the case where the spin and orbital Zeeman splittings cancel each other out in two of the one-particle levels among four. This situation seems to be realized in the recent experiment. Using the Wilson numerical renormalization group, we show that a crossover from the SU(4) to SU(2) Fermi-liquid behavior occurs as magnetic field increases at two impurity-electrons filling. We also find that the quasiparticles are significantly renormalized as the remaining two one-particle levels move away from the Fermi level and are frozen at high magnetic fields. Furthermore, we consider how the singlet ground state evolves during such a crossover. Specifically, we reexamine the SU(N) Kondo singlet for M impurity-electrons filling in the limit of strong exchange interactions. We find that the nondegenerate Fermi-liquid fixed point of Nozières and Blandin can be described as abosonic Perron-Frobenius vector for M composite pairs, each of which consists of one impurity-electron and one conduction-hole. This interpretation in terms of the Perron-Frobenius theorem can also be extended to the Fermi-liquid fixed-point without the SU(N) symmetry.

  20. Kondo Impurities in the Kitaev Spin Liquid: Numerical Renormalization Group Solution and Gauge-Flux-Driven Screening.

    PubMed

    Vojta, Matthias; Mitchell, Andrew K; Zschocke, Fabian

    2016-07-15

    Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit. PMID:27472132

  1. Kondo Impurities in the Kitaev Spin Liquid: Numerical Renormalization Group Solution and Gauge-Flux-Driven Screening

    NASA Astrophysics Data System (ADS)

    Vojta, Matthias; Mitchell, Andrew K.; Zschocke, Fabian

    2016-07-01

    Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.

  2. Non-Kondo-like electronic structure in the correlated rare-earth hexaboride YbB(6).

    PubMed

    Neupane, Madhab; Xu, Su-Yang; Alidoust, Nasser; Bian, Guang; Kim, D J; Liu, Chang; Belopolski, I; Chang, T-R; Jeng, H-T; Durakiewicz, T; Lin, H; Bansil, A; Fisk, Z; Hasan, M Z

    2015-01-01

    We present angle-resolved photoemission studies on the rare-earth-hexaboride YbB(6), which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB(6) exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB(6) has three 2D Dirac cone like surface states enclosing the Kramers's points, while the f orbital that would be relevant for the Kondo mechanism is ∼1  eV below the Fermi level. Our first-principles calculation shows that the topological state that we observe in YbB(6) is due to an inversion between Yb d and B p bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.

  3. Magnetically tunable Kondo-Aharonov-Bohm effect in a triangular quantum dot.

    PubMed

    Kuzmenko, T; Kikoin, K; Avishai, Y

    2006-02-01

    The role of discrete orbital symmetry in mesoscopic physics is manifested in a system consisting of three identical quantum dots forming an equilateral triangle. Under a perpendicular magnetic field, this system demonstrates a unique combination of Kondo and Aharonov-Bohm features due to an interplay between continuous [spin-rotation SU(2)] and discrete (permutation C3v) symmetries, as well as U(1) gauge invariance. The conductance as a function of magnetic flux displays sharp enhancement or complete suppression depending on contact setups.

  4. Vibration-induced Kondo tunneling through metal-organic complexes with even electron occupation number.

    PubMed

    Kikoin, K; Kiselev, M N; Wegewijs, M R

    2006-05-01

    We investigate transport through a mononuclear transition-metal complex with strong tunnel coupling to two electrodes. The ground state of this molecule is a singlet, while the first excited state is a triplet. We show that a modulation of the tunnel-barrier due to a molecular distortion which couples to the tunneling induces a Kondo-effect, provided the discrete vibrational energy compensates the singlet-triplet gap. We discuss the single-phonon and two-phonon-assisted cotunneling and possible experimental realization of the theory.

  5. Many-body breakdown of indirect gap in topological Kondo insulators

    NASA Astrophysics Data System (ADS)

    Wysokiński, Marcin M.; Fabrizio, Michele

    2016-09-01

    We show that the inclusion of nonlocal correlation effects in a variational wave function for the ground state of a topological Anderson lattice Hamiltonian is capable of describing both topologically trivial insulating phases and nontrivial ones characterized by an indirect gap, as well as its closure at the transition into a metallic phase. The method, though applied to an oversimplified model, thus captures the metallic and insulating states that are indeed observed in a variety of Kondo semiconductors, while accounting for topologically nontrivial band structures.

  6. Telmisartan-mediated metabolic profile conferred brain protection in diabetic hypertensive rats as evidenced by magnetic resonance imaging, behavioral studies and histology.

    PubMed

    Younis, Firas M; Blumenthal-Katzir, Tamar; Hollander, Kenneth; Grigoriadis, Nikolaos; Touloumi, Olga; Lagoudakic, Roza; Rosenthal, Talma

    2016-10-15

    Type 2 diabetes and hypertension are associated with cognitive dysfunction that includes pathological changes in brain tissue. It was speculated that the beneficial hypotensive effect of telmisartan, an angiotensin receptor 1 blocker, and its unique hypoglycemic effect due to its PPARγ-activation, could ameliorate the ​ pathological changes in the brain​ that accompany​ these diseases. We examined the effect of telmisartan on brain changes in magnetic resonance imaging (MRI) T2-weighted scans, and behavioral and histological findings in the Cohen-Rosenthal Diabetic Hypertensive (CRDH) rat. Baseline and post-treatment values with telmisartan/vehicle (3 months) of blood pressure, blood glucose levels, behavioral tests, brain MRI scanning and immunohistological staining were obtained. Telmisartan significantly lowered blood pressure and blood glucose levels; induced consistent T2 reduction in specific gray and white regions including hippocampus, corpus callosum, amygdala and cortical regions; and significantly improved performance on behavioral tasks. Immunohistological analysis of the brain revealed significant amelioration of diabetes/hypertension-induced changes in white matter regions and microglia, evidenced by preserved myelin (LBF marker), and improved microglial neuronal markers GFAP, GAP43 and Iba1 expression. In conclusion, the behavioral performance, longitudinal MRI study and histology staining revealed the protective effects of telmisartan on brain microstructure and cognitive function.

  7. Antiferromagnetic Kondo lattice in the layered compound CePd1–xBi₂ and comparison to the superconductor LaPd1–xBi₂

    SciTech Connect

    Han, Fei; Wan, Xiangang; Phelan, Daniel; Stoumpos, Constantinos C.; Sturza, Mihai; Malliakas, Christos D.; Li, Qing'an; Han, Tian-Heng; Zhao, Qingbiao; Chung, Duck Young; Kanatzidis, Mercouri G.

    2015-07-13

    The layered compound CePd1–xBi₂ with the tetragonal ZrCuSi₂-type structure was obtained from excess Bi flux. Magnetic susceptibility data of CePd1–xBi₂ show an antiferromagnetic ordering below 6 K and are anisotropic along the c axis and the ab plane. The anisotropy is attributed to crystal-electric-field (CEF) effects and a CEF model which is able to describe the susceptibility data is given. An enhanced Sommerfeld coefficient γ of 0.191 J mol Ce⁻¹ K⁻² obtained from specific-heat measurement suggests a moderate Kondo effect in CePd1–xBi₂. Other than the antiferromagnetic peak at 6 K, the resistivity curve shows a shoulderlike behavior around 75 K which could be attributed to the interplay between Kondo and CEF effects. Magnetoresistance and Hall-effect measurements suggest that the interplay reconstructs the Fermi-surface topology of CePd1–xBi₂ around 75 K. Electronic structure calculations reveal that the Pd vacancies are important to the magnetic structure and enhance the CEF effects which quench the orbital moment of Ce at low temperatures.

  8. Kondo effect in a carbon nanotube with spin-orbit interaction and valley mixing: A DM-NRG study

    NASA Astrophysics Data System (ADS)

    Mantelli, Davide; Paşcu Moca, Cătălin; Zaránd, Gergely; Grifoni, Milena

    2016-03-01

    We investigate the effects of spin-orbit interaction (SOI) and valley mixing on the transport and dynamical properties of a carbon nanotube (CNT) quantum dot in the Kondo regime. As these perturbations break the pseudo-spin symmetry in the CNT spectrum but preserve time-reversal symmetry, they induce a finite splitting Δ between formerly degenerate Kramers pairs. Correspondingly, a crossover from the SU(4) to the SU(2)-Kondo effect occurs as the strength of these symmetry breaking parameters is varied. Clear signatures of the crossover are discussed both at the level of the spectral function as well as of the conductance. In particular, we demonstrate numerically and support with scaling arguments that the Kondo temperature scales inversely with the splitting Δ in the crossover regime. In presence of a finite magnetic field, time reversal symmetry is also broken. We investigate the effects of both parallel and perpendicular fields (with respect to the tube's axis) and discuss the conditions under which Kondo revivals may be achieved.

  9. Interplay between crystal field splitting and Kondo effect in CeNi9Ge(4-x)Si(x).

    PubMed

    Gold, C; Gross, P; Peyker, L; Eickerling, G; Simeoni, G G; Stockert, O; Kampert, E; Wolff-Fabris, F; Michor, H; Scheidt, E-W

    2012-09-01

    The pseudo-ternary solid solution CeNi(9)Ge(4-x)Si(x) (0 ≤ x ≤ 4) has been investigated by means of x-ray diffraction, magnetic susceptibility, specific heat, electrical resistivity, thermopower and inelastic neutron scattering studies. The isoelectronic substitution of germanium by silicon atoms causes a dramatic change of the relative strength of competing Kondo, RKKY and crystal field (CF) energy scales. The strongest effect is the continuous elevation of the Kondo temperature T(K) from approximately 3.5 K for CeNi(9)Ge(4) to about 70 K for CeNi(9)Si(4). This increase of the Kondo temperature is attended by a change of the CF level scheme of the Ce ions. The interplay of the different energy scales results in an incipient reduction of the ground state degeneracy from an effectively fourfold degenerate non-magnetic Kondo ground state with unusual non-Fermi-liquid features of CeNi(9)Ge(4) to a lower one, followed by an increase towards a sixfold, fully degenerate ground state multiplet in CeNi(9)Si(4) (T(K) ∼ Δ(CF)).

  10. Pressure Dependence Transport Studies of the Possible Charge Kondo Effect in Tl-doped PbTe

    NASA Astrophysics Data System (ADS)

    Kurosaki, Yosuke; Shinagawa, Jun; Matsushita, Yana; Geballe, Ted; Fisher, Ian; Brown, Stuart

    2006-03-01

    Pb1-xTlxTe is noteworthy for a high superconducting transition temperature relative to carrier concentration, as well as normal state properties consistent with a charge-Kondo effect. Recent experiments also demonstrate that the onset of an observable superconducting Tc with Tl concentration at x˜0.3% coincides with features characteristic of charge Kondo [1], including dρ/dT<0 at low temperatures and an unusual linear variation of the resistivity ρ(T)=ρ0+AT at higher temperatures. Together, these observations are consistent with an association between the two phenomena [2]. We report the effect of applied pressures up to P˜1.5GPa on ρ(T), Tc, and the Hall number pH≡RH-1 for x= 0.3%, 0.8%, and 1.3%. Tc is reduced sharply with pressure, dTc/dP=400-500mK/GPa as the low temperature Kondo- like upturn in ρ(T) is weakened. Also, dA/dP<0 and dpH/dP>0. These observations are discussed in the context of the proposed charge-Kondo model for Pb1-xTlxTe. [1] Y. Matsushita, H. Bluhm, T.H. Geballe and I.R. Fisher, Phys.Rev.Lett. 94, 157002(2005).[2] M. Dzero and J. Schmalian, Phys.Rev.Lett. 94, 157003 (2005). This work is supported by NSF frant DMR-0520552.

  11. Breakdown of the Kondo insulating state in SmB6 by introducing Sm vacancies

    NASA Astrophysics Data System (ADS)

    Valentine, Michael E.; Koohpayeh, Seyed; Phelan, W. Adam; McQueen, Tyrel M.; Rosa, Priscila F. S.; Fisk, Zachary; Drichko, Natalia

    2016-08-01

    We explore the stability of the hybridization gap in SmB6 to the presence of a small number of Sm vacancies typical for this material, and demonstrate the extreme fragility of the Kondo insulating state. For the most stoichiometric sample we detect the hybridization gap which appears below 50 K as a depressed electronic Raman intensity below about 30 meV. The spectral weight that shifts to higher frequencies on the opening of the hybridization gap forms two electronic maxima at 100 and 41 meV. We assign these maxima to the excitations between hybridized 4 f -5 d bands using recent band structure calculations. Below 30 K, in-gap exciton modes with long lifetimes protected by the hybridization gap develop at 16-18 meV. With the increase of the number of Sm vacancies the exciton features broaden, evidencing a decrease in the lifetime due to the presence of electronic states in the gap. At a concentration of Sm vacancies of only about 1% the in-gap exciton is completely quenched, and the hybridization gap is not fully opened. We suggest that only the most stoichiometric SmB6 samples possess a bulk gap necessary for the topological Kondo insulator state.

  12. Formation of metallic magnetic clusters in a Kondo-lattice metal: Evidence from an optical study

    PubMed Central

    Kovaleva, N. N.; Kugel, K. I.; Bazhenov, A. V.; Fursova, T. N.; Löser, W.; Xu, Y.; Behr, G.; Kusmartsev, F. V.

    2012-01-01

    Magnetic materials are usually divided into two classes: those with localised magnetic moments, and those with itinerant charge carriers. We present a comprehensive experimental (spectroscopic ellipsomerty) and theoretical study to demonstrate that these two types of magnetism do not only coexist but complement each other in the Kondo-lattice metal, Tb2PdSi3. In this material the itinerant charge carriers interact with large localised magnetic moments of Tb(4f) states, forming complex magnetic lattices at low temperatures, which we associate with self-organisation of magnetic clusters. The formation of magnetic clusters results in low-energy optical spectral weight shifts, which correspond to opening of the pseudogap in the conduction band of the itinerant charge carriers and development of the low- and high-spin intersite electronic transitions. This phenomenon, driven by self-trapping of electrons by magnetic fluctuations, could be common in correlated metals, including besides Kondo-lattice metals, Fe-based and cuprate superconductors. PMID:23189239

  13. Dissipative phases in the one-dimensional Kondo-Heisenberg model

    NASA Astrophysics Data System (ADS)

    Lobos, Alejandro; Cazalilla, Miguel A.; Chudzinski, Piotr

    2012-02-01

    Atomic-sized magnetic structures built on clean metallic surfaces are currently under intense investigation [1]. Besides their potential uses in quantum information storage and processing, these systems allow to ask fundamental questions in condensed matter physics. In particular, the interplay between the Kondo effect (i.e., the screening of the atomic magnetic moment by conduction electrons) and Heisenberg exchange interactions between magnetic impurities has been recently investigated with scanning tunneling microscopy (STM) [2]. Inspired by the above developments, we study an one-dimensional chain of S=1/2 Kondo impurities coupled by anisotropic Heisenberg-Ising exchange and embedded in a two-dimensional metallic substrate. Remarkably, in the case of easy-plane exchange, we find a novel quantum phase exhibiting long-range order at zero temperature. We discuss implications of the existence of this phase for possible experiments. References: [1] R. Wiesendanger, RMP 81, 1495 (2009). [2] P. Wahl et al, PRL 98, 056601 (2007) and references therein.

  14. Magnetic phenomena, ferro and antiferro Kondo, and transport in transition metal break junction nanocontacts

    NASA Astrophysics Data System (ADS)

    Tosatti, Erio

    2009-03-01

    Transport in transition metal break junctions is of particular interest in connection with magnetism, which may be present either in the leads, and/or in bridging magnetic impurities, or else which may emerge spontaneously at the nanocontact, as expected in pristine Pt or Pd.[1] The standard Landauer ballistic conductance across the locally magnetic atomic contact is modified by Kondo phenomena that are predicted using ab initio electronic structure as a starting point, and the numerical renormalization group as a tool. The case of a magnetic impurity in a nonmagnetic contact[2] is shown to illustrate the competition between antiferro and ferro Kondo screening[3] and its effects on conductance. *) Work in collaboration with A. Smogunov, A. Dal Corso, L. De Leo, P. Gentile, M. Fabrizio, P. Lucignano, and R. Mazzarello. [1] A. Delin, et al., Phys. Rev. Lett. 92, 057201 (2004); A. Smogunov et al., Phys. Rev. B78, 014423 (2008). [2] R. Mazzarello, P. Lucignano, A. Smogunov, M. Fabrizio, and E. Tosatti, in preparation [3] P. Gentile, L. De Leo, M. Fabrizio, and E. Tosatti, in preparation

  15. Kondo effect in a neutral and stable all organic radical single molecule break junction

    NASA Astrophysics Data System (ADS)

    Burzuri, Enrique; Gaudenzi, Rocco; Frisenda, Riccardo; Franco, Carlos; Mas-Torrent, Marta; Rovira, Concepcio; Veciana, Jaume; Alcon, Isaac; Bromley, Stefan T.; van der Zant, Herre S. J.

    Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin-orbit coupling makes organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. We show that the paramagnetism of the PTM radical molecule, in the shape of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical specie. We further study polyradical systems, where several unpaired spins interact in the same molecule. This work was supported by the EU FP7 program through project 618082 ACMOL and ERC grant advanced Mols@Mols. It was also supported by the Dutch funding organization NWO (VENI).

  16. Influence of Rashba spin-orbit coupling on the Kondo effect

    NASA Astrophysics Data System (ADS)

    Wong, Arturo; Ulloa, Sergio E.; Sandler, Nancy; Ingersent, Kevin

    2016-02-01

    An Anderson model for a magnetic impurity in a two-dimensional electron gas with bulk Rashba spin-orbit interaction is solved using the numerical renormalization group under two different experimental scenarios. For a fixed Fermi energy, the Kondo temperature TK varies weakly with Rashba coupling λR, as reported previously. If instead the band filling is low and held constant, increasing λR can drive the system into a helical regime with exponential enhancement of TK. Under either scenario, thermodynamic properties at low temperatures T exhibit the same dependencies on T /TK as are found for λR=0 . Unlike the conventional Kondo effect, however, the impurity exhibits static spin correlations with conduction electrons of nonzero orbital angular momentum about the impurity site. We also consider a magnetic field that Zeeman splits the conduction band but not the impurity level, an effective picture that arises under a proposed route to access the helical regime in a driven system. The impurity contribution to the system's ground-state angular momentum is found to be a universal function of the ratio of the Zeeman energy to a temperature scale that is not TK (as would be the case in a magnetic field that couples directly to the impurity spin), but rather is proportional to TK divided by the impurity hybridization width. This universal scaling is explained via a perturbative treatment of field-induced changes in the electronic density of states.

  17. Magnetotransport in (Ce1-xNdx)Cu6 Kondo alloys

    NASA Astrophysics Data System (ADS)

    Strydom, André M.; du Plessis, Paul de V.

    1999-03-01

    The results of electrical resistivity ρ(T) and magnetoresistivity MR(T, B) for $1.5 \\le T \\le 580$Kondo lattice is characterized through coherence effects in ρ(T) at low temperatures. The ρ(T) data above room temperature are used to resolve the electron-phonon scattering, and it is indicated that the single-ion Kondo interaction dominates both ρ(T) and MR(B) for a wide range of intermediate Ce concentrations. Based on this, the MR(B) data for different isotherms and alloy compositions are analysed according to the Bethe- ansatz description. We also discuss the observed deviations of our data from the preceding theoretical description due to the onset of magnetic order in alloys with high Nd content, and to phase coherence at low temperatures.

  18. Heavy-fermion quantum criticality and destruction of the Kondo effect in a nickel oxypnictide.

    PubMed

    Luo, Yongkang; Pourovskii, Leonid; Rowley, S E; Li, Yuke; Feng, Chunmu; Georges, Antoine; Dai, Jianhui; Cao, Guanghan; Xu, Zhu'an; Si, Qimiao; Ong, N P

    2014-08-01

    A quantum critical point arises at a continuous transformation between distinct phases of matter at zero temperature. Studies in antiferromagnetic heavy-fermion materials have revealed that quantum criticality has several classes, with an unconventional type that involves a critical destruction of the Kondo entanglement. To understand such varieties, it is important to extend the materials basis beyond the usual setting of intermetallic compounds. Here we show that a nickel oxypnictide, CeNiAsO, exhibits a heavy-fermion antiferromagnetic quantum critical point as a function of either pressure or P/As substitution. At the quantum critical point, non-Fermi-liquid behaviour appears, which is accompanied by a divergent effective carrier mass. Across the quantum critical point, the low-temperature Hall coefficient undergoes a rapid sign change, suggesting a sudden jump of the Fermi surface and a destruction of the Kondo effect. Our results imply that the enormous materials basis for the oxypnictides, which has been so crucial in the search for high-temperature superconductivity, will also play a vital role in the effort to establish the universality classes of quantum criticality in strongly correlated electron systems. PMID:24859644

  19. Wigner and Kondo physics in quantum point contacts revealed by scanning gate microscopy.

    PubMed

    Brun, B; Martins, F; Faniel, S; Hackens, B; Bachelier, G; Cavanna, A; Ulysse, C; Ouerghi, A; Gennser, U; Mailly, D; Huant, S; Bayot, V; Sanquer, M; Sellier, H

    2014-06-30

    Quantum point contacts exhibit mysterious conductance anomalies in addition to well-known conductance plateaus at multiples of 2e(2)/h. These 0.7 and zero-bias anomalies have been intensively studied, but their microscopic origin in terms of many-body effects is still highly debated. Here we use the charged tip of a scanning gate microscope to tune in situ the electrostatic potential of the point contact. While sweeping the tip distance, we observe repetitive splittings of the zero-bias anomaly, correlated with simultaneous appearances of the 0.7 anomaly. We interpret this behaviour in terms of alternating equilibrium and non-equilibrium Kondo screenings of different spin states localized in the channel. These alternating Kondo effects point towards the presence of a Wigner crystal containing several charges with different parities. Indeed, simulations show that the electron density in the channel is low enough to reach one-dimensional Wigner crystallization over a size controlled by the tip position.

  20. Magnetic properties of Ce{sup 3+} in Pb{sub 1{minus}x}Ce{sub x}Se: Kondo and crystal-field effect

    SciTech Connect

    Gratens, X.; Charar, S.; Averous, M.; Isber, S.; Deportes, J.; Golacki, Z.

    1997-10-01

    Electron paramagnetic resonance (EPR) experiments were performed on a Pb{sub 1{minus}x}Ce{sub x}Se crystal at liquid-helium temperatures and show very clearly that the doublet {Gamma}{sub 7} is the ground state for cerium ions. The cubic symmetry is shown and the effective Land{acute e} factor for the Ce{sup 3+} is determined to be 1.354{plus_minus}0.003. An orbital reduction factor is introduced to explain the g experimental value. High-field magnetization results are in good agreement with the EPR results. The nominal Ce composition in PbSe deduced from saturation of the magnetization, x=0.0405{plus_minus}0.0003, is very closed to the value determined by microprobe analysis (x=0.04). At 1.5 K, an antiferromagnetic interaction between the nearest-neighbor cerium atoms is found, J{sub ex}/k{sub B}={minus}0.715thinspK. The low-field magnetic-susceptibility results show that the magnetic moment of cerium impurities is strongly temperature dependent, explained by the presence of the crystal-field effect and the Kondo effect. {copyright} {ital 1997} {ital The American Physical Society}

  1. Kondo lattice mixed valence behavior in the Ce(SnxPb1 - x)3 system

    NASA Astrophysics Data System (ADS)

    Teter, J.; Freitag, R.; Maury*, A.; Crow, J. E.; Mihalisin, T.

    1982-11-01

    Measurements of the electrical resistivity versus x and temperature T, for 1.5≤T≤300 K for the fcc system Ce(SnxPb1-x)3 are reported. CeSn3 has been shown to be a strongly mixed valent system with an average occupation number of the Ce 4f level nf of ˜0.4 at low temperatures. The electrical resistivity for Ce(SnxPb1-x)3 is compared to that obtained for other Ce based mixed valent-trivalent systems and to the predictions of the Newns and Hewson theory. These comparisons suggest that Ce(SnxPb1-x)3 is mixed valent for x≳0.5 and the scaling of the resistivity supports the previous result that CeSn3 is strong mixed valent with nf≂0.4.

  2. Behaviorism

    ERIC Educational Resources Information Center

    Moore, J.

    2011-01-01

    Early forms of psychology assumed that mental life was the appropriate subject matter for psychology, and introspection was an appropriate method to engage that subject matter. In 1913, John B. Watson proposed an alternative: classical S-R behaviorism. According to Watson, behavior was a subject matter in its own right, to be studied by the…

  3. Pressure-tuned quantum criticality in the antiferromagnetic Kondo semimetal CeNi2–δAs2

    SciTech Connect

    Luo, Yongkang; Ronning, F.; Wakeham, N.; Lu, Xin; Park, Tuson; Xu, Z. -A.; Thompson, J. D.

    2015-10-19

    The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi2–δAs2 (δ ≈ 0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of ~0.032 e/formular unit in CeNi2–δAs2 leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo-lattice state with decreasing temperature. Here, the small carrier density and associated semimetallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raises the specter of the Nozières exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening.

  4. Tunneling and Josephson effects in odd-frequency superconductor junctions: A study on multichannel Kondo chain

    NASA Astrophysics Data System (ADS)

    Hoshino, Shintaro; Yada, Keiji; Tanaka, Yukio

    2016-06-01

    Junction systems of odd-frequency (OF) superconductors are investigated based on a mean-field Hamiltonian formalism. One-dimensional two-channel Kondo lattice (TCKL) is taken as a concrete example of OF superconductors. Properties of normal and Andreev reflections are examined in a normal metal/superconductor junction. Unlike conventional superconductors, normal reflection is always present due to the normal self energy that necessarily appears in the present OF pairing state. The conductance reflects the difference between repulsive and attractive potentials located at the interface, which is in contrast with the preexisting superconducting junctions. Josephson junction is also constructed by connecting TCKL with the other types of superconductors. The results can be understood from symmetry of the induced Cooper pairs at the edge in the presence of spin/orbital symmetry breaking. It has also been demonstrated that the symmetry argument for Cooper pairs is useful in explaining Meissner response in bulk.

  5. Quantum Phase Transition and Protected Ideal Transport in a Kondo Chain.

    PubMed

    Tsvelik, A M; Yevtushenko, O M

    2015-11-20

    We study the low energy physics of a Kondo chain where electrons from a one-dimensional band interact with magnetic moments via an anisotropic exchange interaction. It is demonstrated that the anisotropy gives rise to two different phases which are separated by a quantum phase transition. In the phase with easy plane anisotropy, Z_{2} symmetry between sectors with different helicity of the electrons is broken. As a result, localization effects are suppressed and the dc transport acquires (partial) symmetry protection. This effect is similar to the protection of the edge transport in time-reversal invariant topological insulators. The phase with easy axis anisotropy corresponds to the Tomonaga-Luttinger liquid with a pronounced spin-charge separation. The slow charge density wave modes have no protection against localization.

  6. Low energy properties of the Kondo chain in the RKKY regime

    DOE PAGES

    D. H. Schimmel; Tsvelik, A. M.; Yevtushenko, O. M.

    2016-05-03

    We study the Kondo chain in the regime of high spin concentration where the low energy physics is dominated by the Ruderman–Kittel–Kasuya–Yosida interaction. As has been recently shown (Tsvelik and Yevtushenko 2015 Phys. Rev. Lett. 115 216402), this model has two phases with drastically different transport properties depending on the anisotropy of the exchange interaction. In particular, the helical symmetry of the fermions is spontaneously broken when the anisotropy is of the easy plane type. This leads to a parametrical suppression of the localization effects. In the present paper we substantially extend the previous theory, in particular, by analyzing amore » competition of forward- and backward- scattering, including into the theory short range electron interactions and calculating spin correlation functions. In conclusion, we discuss applicability of our theory and possible experiments which could support the theoretical findings.« less

  7. Kondo effect in the helical edge liquid of the quantum spin Hall state.

    PubMed

    Maciejko, Joseph; Liu, Chaoxing; Oreg, Yuval; Qi, Xiao-Liang; Wu, Congjun; Zhang, Shou-Cheng

    2009-06-26

    Following the recent observation of the quantum spin Hall (QSH) effect in HgTe quantum wells, an important issue is to understand the effect of impurities on transport in the QSH regime. Using linear response and renormalization group methods, we calculate the edge conductance of a QSH insulator as a function of temperature in the presence of a magnetic impurity. At high temperatures, Kondo and/or two-particle scattering give rise to a logarithmic temperature dependence. At low temperatures, for weak Coulomb interactions in the edge liquid, the conductance is restored to unitarity with unusual power laws characteristic of a "local helical liquid," while for strong interactions, transport proceeds by weak tunneling through the impurity where only half an electron charge is transferred in each tunneling event. PMID:19659109

  8. Quantum phase transition and protected ideal transport in a Kondo chain

    SciTech Connect

    Tsvelik, A. M.; Yevtushenko, O. M.

    2015-11-30

    We study the low energy physics of a Kondo chain where electrons from a one-dimensional band interact with magnetic moments via an anisotropic exchange interaction. It is demonstrated that the anisotropy gives rise to two different phases which are separated by a quantum phase transition. In the phase with easy plane anisotropy, Z2 symmetry between sectors with different helicity of the electrons is broken. As a result, localization effects are suppressed and the dc transport acquires (partial) symmetry protection. This effect is similar to the protection of the edge transport in time-reversal invariant topological insulators. The phase with easy axis anisotropy corresponds to the Tomonaga-Luttinger liquid with a pronounced spin-charge separation. The slow charge density wave modes have no protection against localizatioin.

  9. Low energy properties of the Kondo chain in the RKKY regime

    NASA Astrophysics Data System (ADS)

    Schimmel, D. H.; Tsvelik, A. M.; Yevtushenko, O. M.

    2016-05-01

    We study the Kondo chain in the regime of high spin concentration where the low energy physics is dominated by the Ruderman-Kittel-Kasuya-Yosida interaction. As has been recently shown (Tsvelik and Yevtushenko 2015 Phys. Rev. Lett. 115 216402), this model has two phases with drastically different transport properties depending on the anisotropy of the exchange interaction. In particular, the helical symmetry of the fermions is spontaneously broken when the anisotropy is of the easy plane type. This leads to a parametrical suppression of the localization effects. In the present paper we substantially extend the previous theory, in particular, by analyzing a competition of forward- and backward- scattering, including into the theory short range electron interactions and calculating spin correlation functions. We discuss applicability of our theory and possible experiments which could support the theoretical findings.

  10. Quantum phase transition and protected ideal transport in a Kondo chain

    DOE PAGES

    Tsvelik, A. M.; Yevtushenko, O. M.

    2015-11-30

    We study the low energy physics of a Kondo chain where electrons from a one-dimensional band interact with magnetic moments via an anisotropic exchange interaction. It is demonstrated that the anisotropy gives rise to two different phases which are separated by a quantum phase transition. In the phase with easy plane anisotropy, Z2 symmetry between sectors with different helicity of the electrons is broken. As a result, localization effects are suppressed and the dc transport acquires (partial) symmetry protection. This effect is similar to the protection of the edge transport in time-reversal invariant topological insulators. The phase with easy axismore » anisotropy corresponds to the Tomonaga-Luttinger liquid with a pronounced spin-charge separation. The slow charge density wave modes have no protection against localizatioin.« less

  11. Kondo effect and thermoelectric transport in CePd3Be x.

    PubMed

    Gumeniuk, Roman; Schnelle, Walter; Kvashnina, Kristina O; Leithe-Jasper, Andreas

    2016-04-27

    The physical properties of the series CePd3Be(x) (0 ≤ x ≤ 0.47) have been studied. Introducing Be into CePd3 results in a drastic reduction of the Seebeck coefficient from 100 μV K(-1) at 300 K to  -2 μV K(-1), respectively. Paramagnetism of Ce(3+) free ions and metallic conduction dominate the physical properties. A structural transition at x  =  0.25 is accompanied by a significant lowering of the Kondo temperature and leads to a successive suppression of the thermoelectric performance of CePd3Be(x) with increasing x. PMID:27009024

  12. Spin-orbital and spin Kondo effects in parallel coupled quantum dots

    NASA Astrophysics Data System (ADS)

    Krychowski, D.; Lipiński, S.

    2016-02-01

    Strong electron correlations and interference effects are discussed in parallel-coupled single-level or orbitally doubly degenerate quantum dots. The finite-U mean-field slave boson approach is used to study many-body effects. The analysis is carried out in a wide range of parameter space including both atomic-like and molecular-like Kondo regimes and taking into account various perturbations, like interdot tunneling, interdot interaction, mixing of the electrode channels, and exchange interaction. We also discuss the influence of singularities of electronic structure and the impact of polarization of electrodes. Special attention is paid to potential spintronic applications of these systems showing how current polarization can be controlled by adjusting interference conditions and correlations by gate voltage. Simple proposals of double dot spin valve and bipolar electrically tunable spin filter are presented.

  13. Proximity effect induced by Kondo interaction in a network composed of YBCO and spin density wave

    NASA Astrophysics Data System (ADS)

    Maity, S.; Ghosh, Ajay Kumar

    2015-10-01

    The possibility of the proximity effect mediated by Kondo interaction in YBCO embedded in system of diluted magnetic spin ordering has been studied. An YBCO sample is selected in which both metal to insulator transition and superconducting state exist in the different ranges of temperature. The intergranular network of the bulk Y-123 has been modified by the inclusion of YMnO3 which has a well defined magnetic structure depending on temperature. The current-voltage measurements have been carried out in pure Y-123 at several temperatures. At the same set of temperatures the current-voltage curves in presence of YMnO3 have been studied. The role of the diluted spin magnetic ordering in tuning proximity effect and conduction property in binary systems is associated with reduced coherence length in the normal region.

  14. Non-universal weak antilocalization effect in cubic topological Kondo insulators

    NASA Astrophysics Data System (ADS)

    Dzero, Maxim; Vavilov, Maxim; Kechedzhi, Kostyantin; Galitski, Victor

    In this talk we present the results of our study of the quantum correction to conductivity on the surface of cubic topological Kondo insulators with multiple Dirac bands. We considered the model of time-reversal invariant disorder which induces the scattering of the electrons within the Dirac bands as well as between the bands. When only intraband scattering is present we found three long-range diffusion modes leading to weak antilocalization correction to conductivity which remains independent of the microscopic details such as Fermi velocities and relaxation times. Interband scattering gaps out two diffusion modes leaving only one long-range mode. Depending on the value of the phase coherence time, either three or only one long-range diffusion modes contribute to weak localization correction rendering the quantum correction to conductivity non-universal.

  15. Foundations of heavy-fermion superconductivity: lattice Kondo effect and Mott physics.

    PubMed

    Steglich, Frank; Wirth, Steffen

    2016-08-01

    This article overviews the development of heavy-fermion superconductivity, notably in such rare-earth-based intermetallic compounds which behave as Kondo-lattice systems. Heavy-fermion superconductivity is of unconventional nature in the sense that it is not mediated by electron-phonon coupling. Rather, in most cases the attractive interaction between charge carriers is apparently magnetic in origin. Fluctuations associated with an antiferromagnetic (AF) quantum critical point (QCP) play a major role. The first heavy-fermion superconductor CeCu2Si2 turned out to be the prototype of a larger group of materials for which the underlying, often pressure-induced, AF QCP is likely to be of a three-dimensional (3D) spin-density-wave (SDW) variety. For UBe13, the second heavy-fermion superconductor, a magnetic-field-induced 3D SDW QCP inside the superconducting phase can be conjectured. Such a 'conventional', itinerant QCP can be well understood within Landau's paradigm of order-parameter fluctuations. In contrast, the low-temperature normal-state properties of a few heavy-fermion superconductors are at odds with the Landau framework. They are characterized by an 'unconventional', local QCP which may be considered a zero-temperature 4 f-orbital selective Mott transition. Here, as concluded for YbRh2Si2, the breakdown of the Kondo effect concurring with the AF instability gives rise to an abrupt change of the Fermi surface. Very recently, superconductivity was discovered for this compound at ultra-low temperatures. Therefore, YbRh2Si2 along with CeRhIn5 under pressure provide a natural link between the large group of about fifty low-temperature heavy-fermion superconductors and other families of unconventional superconductors with substantially higher T c, e.g. the doped Mott insulators of the perovskite-type cuprates and the organic charge-transfer salts.

  16. Foundations of heavy-fermion superconductivity: lattice Kondo effect and Mott physics

    NASA Astrophysics Data System (ADS)

    Steglich, Frank; Wirth, Steffen

    2016-08-01

    This article overviews the development of heavy-fermion superconductivity, notably in such rare-earth-based intermetallic compounds which behave as Kondo-lattice systems. Heavy-fermion superconductivity is of unconventional nature in the sense that it is not mediated by electron-phonon coupling. Rather, in most cases the attractive interaction between charge carriers is apparently magnetic in origin. Fluctuations associated with an antiferromagnetic (AF) quantum critical point (QCP) play a major role. The first heavy-fermion superconductor CeCu2Si2 turned out to be the prototype of a larger group of materials for which the underlying, often pressure-induced, AF QCP is likely to be of a three-dimensional (3D) spin-density-wave (SDW) variety. For UBe13, the second heavy-fermion superconductor, a magnetic-field-induced 3D SDW QCP inside the superconducting phase can be conjectured. Such a ‘conventional’, itinerant QCP can be well understood within Landau’s paradigm of order-parameter fluctuations. In contrast, the low-temperature normal-state properties of a few heavy-fermion superconductors are at odds with the Landau framework. They are characterized by an ‘unconventional’, local QCP which may be considered a zero-temperature 4 f-orbital selective Mott transition. Here, as concluded for YbRh2Si2, the breakdown of the Kondo effect concurring with the AF instability gives rise to an abrupt change of the Fermi surface. Very recently, superconductivity was discovered for this compound at ultra-low temperatures. Therefore, YbRh2Si2 along with CeRhIn5 under pressure provide a natural link between the large group of about fifty low-temperature heavy-fermion superconductors and other families of unconventional superconductors with substantially higher T c, e.g. the doped Mott insulators of the perovskite-type cuprates and the organic charge-transfer salts.

  17. Foundations of heavy-fermion superconductivity: lattice Kondo effect and Mott physics.

    PubMed

    Steglich, Frank; Wirth, Steffen

    2016-08-01

    This article overviews the development of heavy-fermion superconductivity, notably in such rare-earth-based intermetallic compounds which behave as Kondo-lattice systems. Heavy-fermion superconductivity is of unconventional nature in the sense that it is not mediated by electron-phonon coupling. Rather, in most cases the attractive interaction between charge carriers is apparently magnetic in origin. Fluctuations associated with an antiferromagnetic (AF) quantum critical point (QCP) play a major role. The first heavy-fermion superconductor CeCu2Si2 turned out to be the prototype of a larger group of materials for which the underlying, often pressure-induced, AF QCP is likely to be of a three-dimensional (3D) spin-density-wave (SDW) variety. For UBe13, the second heavy-fermion superconductor, a magnetic-field-induced 3D SDW QCP inside the superconducting phase can be conjectured. Such a 'conventional', itinerant QCP can be well understood within Landau's paradigm of order-parameter fluctuations. In contrast, the low-temperature normal-state properties of a few heavy-fermion superconductors are at odds with the Landau framework. They are characterized by an 'unconventional', local QCP which may be considered a zero-temperature 4 f-orbital selective Mott transition. Here, as concluded for YbRh2Si2, the breakdown of the Kondo effect concurring with the AF instability gives rise to an abrupt change of the Fermi surface. Very recently, superconductivity was discovered for this compound at ultra-low temperatures. Therefore, YbRh2Si2 along with CeRhIn5 under pressure provide a natural link between the large group of about fifty low-temperature heavy-fermion superconductors and other families of unconventional superconductors with substantially higher T c, e.g. the doped Mott insulators of the perovskite-type cuprates and the organic charge-transfer salts. PMID:27376190

  18. Hybridization behavior of mixed DNA/alkylthiol monolayers on gold: characterization by surface plasmon resonance and 32P radiometric assay.

    PubMed

    Gong, Ping; Lee, Chi-Ying; Gamble, Lara J; Castner, David G; Grainger, David W

    2006-05-15

    Nucleic acid assay from a complex biological milieu is attractive but currently difficult and far from routine. In this study, DNA hybridization from serum dilutions into mixed DNA/mercaptoundecanol (MCU) adlayers on gold was monitored by surface plasmon resonance (SPR). Immobilized DNA probe and hybridized target densities on these surfaces were quantified using 32P-radiometric assays as a function of MCU diluent exposure. SPR surface capture results correlated with radiometric analysis for hybridization performance, demonstrating a maximum DNA hybridization on DNA/MCU mixed adlayers. The maximum target surface capture produced by MCU addition to the DNA probe layer correlates with structural and conformational data on identical mixed DNA/MCU adlayers on gold derived from XPS, NEXAFS, and fluorescence intensity measurements reported in a related study (Lee, C.-Y.; Gong, P.; Harbers, G. M.; Grainger, D. W.; Castner, D. G.; Gamble, L. J. Anal. Chem. 2006, 78, 3316-3325.). MCU addition into the DNA adlayer on gold also improved surface resistance to both nonspecific DNA and serum protein adsorption. Target DNA hybridization from serum dilutions was monitored with SPR on the optimally mixed DNA/MCU adlayers. Both hybridization kinetics and efficiency were strongly affected by nonspecific protein adsorption from a complex milieu even at a minimal serum concentration (e.g., 1%). No target hybridization was detected in SPR assays from serum concentrations above 30%, indicating nonspecific protein adsorption interference of DNA capture and hybridization from complex milieu. Removal of nonsignal proteins from nucleic acid targets prior to assay represents a significant issue for direct sample-to-assay nucleic acid diagnostics from food, blood, tissue, PCR mixtures, and many other biologically complex sample formats. PMID:16689533

  19. Behavioral, histological, and ex vivo magnetic resonance imaging assessment of graded contusion spinal cord injury in mice.

    PubMed

    Nishi, Rebecca A; Liu, Hongli; Chu, Yong; Hamamura, Mark; Su, Min-Ying; Nalcioglu, Orhan; Anderson, Aileen J

    2007-04-01

    This study characterized the Infinite Horizon (IH) Impactor for use in mouse models of contusion spinal cord injury (SCI), and investigated the feasibility and reliability of using magnetic resonance imaging (MRI) as a method to accurately measure lesion volume after mouse contusion SCI. Eight-week-old female C57Bl/6 mice received a mild (30 kilodyne), moderate (50 kilodyne), or severe (70 kilodyne) contusion injury at the T9 vertebral level. Uninjured control mice received a T9 laminectomy only. Functional recovery was assessed using the Basso, Beattie, Bresnahan (BBB) and Basso Mouse Scale (BMS) open-field locomotor rating scales. Next, 4% paraformaldehyde-perfused spinal cords were collected between the T6 and T12 spinal roots, and stored in phosphate-buffered saline (PBS) at 4 degrees C until MRI analysis. MRI lesion volumes were determined using T1-weighted images on a 7-Tesla MRI. Histology was performed on 20-microm polyester wax-embedded sections processed from the same spinal cords for stereological determination of fibronectin lesion volume and myelin basic protein spared white matter volume. Area of spared white matter at the epicenter was also analyzed. The results demonstrated that the IH Impactor produced precise, graded contusion SCI in mice. Lesion volumes were positively correlated with force of impact, and negatively correlated with spared white matter and functional recovery. Additionally, similar lesion volumes were detected using fibronectin staining and MRI analysis, although MRI may be more sensitive for milder injuries. These results give researchers more options in how to analyze spinal cord injuries in animal models.

  20. Two-Channel Kondo Physics due to As Vacancies in the Layered Compound ZrAs_{1.58}Se_{0.39}.

    PubMed

    Cichorek, T; Bochenek, L; Schmidt, M; Czulucki, A; Auffermann, G; Kniep, R; Niewa, R; Steglich, F; Kirchner, S

    2016-09-01

    We address the origin of the magnetic-field-independent -|A|T^{1/2} term observed in the low-temperature resistivity of several As-based metallic systems of the PbFCl structure type. For the layered compound ZrAs_{1.58}Se_{0.39}, we show that vacancies in the square nets of As give rise to the low-temperature transport anomaly over a wide temperature regime of almost two decades in temperature. This low-temperature behavior is in line with the nonmagnetic version of the two-channel Kondo effect, whose origin we ascribe to a dynamic Jahn-Teller effect operating at the vacancy-carrying As layer with a C_{4} symmetry. The pair-breaking nature of the dynamical defects in the square nets of As explains the low superconducting transition temperature T_{c}≈0.14  K of ZrAs_{1.58}Se_{0.39} compared to the free-of-vacancies homologue ZrP_{1.54}S_{0.46} (T_{c}≈3.7  K). Our findings should be relevant to a wide class of metals with disordered pnictogen layers. PMID:27636484

  1. Two-Channel Kondo Physics due to As Vacancies in the Layered Compound ZrAs_{1.58}Se_{0.39}.

    PubMed

    Cichorek, T; Bochenek, L; Schmidt, M; Czulucki, A; Auffermann, G; Kniep, R; Niewa, R; Steglich, F; Kirchner, S

    2016-09-01

    We address the origin of the magnetic-field-independent -|A|T^{1/2} term observed in the low-temperature resistivity of several As-based metallic systems of the PbFCl structure type. For the layered compound ZrAs_{1.58}Se_{0.39}, we show that vacancies in the square nets of As give rise to the low-temperature transport anomaly over a wide temperature regime of almost two decades in temperature. This low-temperature behavior is in line with the nonmagnetic version of the two-channel Kondo effect, whose origin we ascribe to a dynamic Jahn-Teller effect operating at the vacancy-carrying As layer with a C_{4} symmetry. The pair-breaking nature of the dynamical defects in the square nets of As explains the low superconducting transition temperature T_{c}≈0.14  K of ZrAs_{1.58}Se_{0.39} compared to the free-of-vacancies homologue ZrP_{1.54}S_{0.46} (T_{c}≈3.7  K). Our findings should be relevant to a wide class of metals with disordered pnictogen layers.

  2. Two-Channel Kondo Physics due to As Vacancies in the Layered Compound ZrAs1.58 Se0.39

    NASA Astrophysics Data System (ADS)

    Cichorek, T.; Bochenek, L.; Schmidt, M.; Czulucki, A.; Auffermann, G.; Kniep, R.; Niewa, R.; Steglich, F.; Kirchner, S.

    2016-09-01

    We address the origin of the magnetic-field-independent -|A |T1 /2 term observed in the low-temperature resistivity of several As-based metallic systems of the PbFCl structure type. For the layered compound ZrAs1.58 Se0.39 , we show that vacancies in the square nets of As give rise to the low-temperature transport anomaly over a wide temperature regime of almost two decades in temperature. This low-temperature behavior is in line with the nonmagnetic version of the two-channel Kondo effect, whose origin we ascribe to a dynamic Jahn-Teller effect operating at the vacancy-carrying As layer with a C4 symmetry. The pair-breaking nature of the dynamical defects in the square nets of As explains the low superconducting transition temperature Tc≈0.14 K of ZrAs1.58 Se0.39 compared to the free-of-vacancies homologue ZrP1.54 S0.46 (Tc≈3.7 K ). Our findings should be relevant to a wide class of metals with disordered pnictogen layers.

  3. Collective behavior of an ensemble of forced duffing oscillators near the 1{vert_ellipsis}1 resonance. Revision 1

    SciTech Connect

    Sen, T.; Ellison, J.; Kauffmann, S.

    1994-07-01

    Preserving the beam size (or equivalently the emittance) is a primary aim of accelerator physics. Here we study the effect on the emittance of power supply ripple in the guiding magnetic fields. The collective behavior of forced Duffing oscillators is the natural model to understand this phenomenon. We consider the case when the external frequency is near the linearized natural frequency and nonlinearity and forcing are small. The method of averaging reduces the problem to an autonomous system. A coarse grained long time limit of the phase space density and the rate of approach to this limit are discussed in terms of the autonomous system. We find the frequencies which lead to the largest emittance growth in three different forcing regimes (weak, moderate and relatively large) and also characterize the dependence of emittance growth on forcing amplitude in these regimes.

  4. Non-fermi liquid and spin-glass behavior of the Sc{sub 1-x}U{sub x}Pd{sub 3} system

    SciTech Connect

    Gajewski, D.A.; Allenspach, P.; Seaman, C.L.; Maple, M.B. |

    1993-09-01

    Previous electrical resistivity {rho}T, magnetic susceptibility {chi}T, and specific heat C(T) measurements on the Y{sub 1-x}U{sub x}Pd{sub 3} system have revealed Kondo behavior for 0 < {times} < 0.2 and spin-glass-like behavior for 0.3 < {times} < 0.5. The Kondo behavior is unusual and characterized by non-Fermi liquid behavior at low temperatures T {much_lt} T{sub K}, where T{sub K} is the Kondo temperature: {rho}T/{rho}(0) {approximately} 1 {minus} T/(aT{sub K}), and C(T)/T {approximately} 1 {minus} (1/T{sub K})1nT with evidence for a finite T = 0 residual entropy S(0) = (R/2)1n(2). We report measurements of {rho}T, {chi}T, and C(T) on the Sc{sub 1-x}U{sub x}Pd{sub 3} system which reveal similar Kondo, non-Fermi liquid, and spin-glass behaviors.

  5. Consistent bosonization-debosonization. II. The two-lead Kondo problem and the fate of its nonequilibrium Toulouse point

    NASA Astrophysics Data System (ADS)

    Bolech, C. J.; Shah, Nayana

    2016-02-01

    Following the development of a scheme to bosonize and debosonize consistently [N. Shah and C. J. Bolech, Phys. Rev. B 93, 085440 (2016), 10.1103/PhysRevB.93.085440], we present in detail the Toulouse-point analytic solution of the two-lead Kondo junction model. The existence and location of the solvable point is not modified, but the calculational methodology and the final expressions for observable quantities change markedly as compared to the existent results. This solvable point is one of the remarkably few exact results for nonequilibrium transport in correlated systems. It yields relatively simple analytical expressions for the current in the full range of temperature, magnetic field, and voltage. It also shows precisely, within the limitations of the Toulouse fine-tuning, how the transport evolves depending on the relative strengths of interlead and intralead Kondo exchange couplings ranging from weak to strong. Thus its improved understanding is an important stepping stone for future research.

  6. Transport properties and Kondo correlations in nanostructures: Time-dependent DMRG method applied to quantum dots coupled to Wilson chains

    SciTech Connect

    Dias Da Silva, Luis G; Heidrich-Meisner, Fabian; Feiguin, Adrian E; Busser, C. A.; Martins, G. B.; Anda, E. V.; Dagotto, Elbio R

    2008-01-01

    We apply the adaptive time-dependent density-matrix renormalization-group method tDMRG to the study of transport properties of quantum-dot systems connected to metallic leads. Finite-size effects make the usual tDMRG description of the Kondo regime a numerically demanding task. We show that such effects can be attenuated by describing the leads by Wilson chains, in which the hopping matrix elements decay exponentially away from the impurity tn n/2. For a given system size and in the linear-response regime, results for 1 show several improvements over the undamped =1 case: perfect conductance is obtained deeper in the strongly interacting regime and current plateaus remain well defined for longer time scales. Similar improvements were obtained in the finite-bias regime up to bias voltages of the order of the Kondo temperature. These results show that with the proposed modification, the tDMRG characterization of Kondo correlations in the transport properties can be substantially improved, while it turns out to be sufficient to work with much smaller system sizes. We discuss the numerical cost of this approach with respect to the necessary system sizes and the entanglement growth during the time evolution.

  7. Non-Kondo-like electronic structure in the correlated rare-earth hexaboride YbB6

    DOE PAGES

    Neupane, Madhab; Xu, Su -Yang; Alidoust, Nasser; Bian, Guang; Kim, D. J.; Liu, Chang; Belopolski, I.; Chang, T. -R.; Jeng, H. -T.; Durakiewicz, T.; et al

    2015-01-07

    Here, we present angle-resolved photoemission studies on the rare-earth-hexaboride YbB6, which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB6 exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB6 has three 2D Dirac cone like surface states enclosing the Kramers’s points, while the f orbital that would be relevant for the Kondo mechanism is ~1 eV below the Fermi level. Our first-principles calculation shows that the topological state that we observe inmore » YbB6 is due to an inversion between Yb d and B p bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.« less

  8. Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect

    NASA Astrophysics Data System (ADS)

    Du, Shixuan

    Control over charge and spin states at the single molecule level is crucial not only for a fundamental understanding of charge and spin interactions but also represents a prerequisite for development of molecular electronics and spintronics. In this talk, I will talk about the extended spin distribution in space beyond the central Mn ion, and onto the non-magnetic constituent atoms of the MnPc molecule. This extended spin distribution results in an extended Kondo effect, which can be explained by spin polarization induced by symmetry breaking of the molecular framework, as confirmed by DFT calculations. Measuring the evolution of the Kondo splitting with applied magnetic fields at different atomic sites, we find a spatial variation of the g-factor within a single molecule for the first time. The existence of atomic site-dependent g-factors can be attributed to specific molecular orbitals distributed over the entire molecule. This work not only open up a new opportunity for quantum information recording, but also provide a new route to explore the internal electronic and spin structure of complex molecules, hard to achieve otherwise. (L. W. Liu et al., Phys. Rev. Lett. 2015, 114, 126601. In collaboration with Liwei Liu, Kai Yang, Yuhang Jiang, Li Gao, Qi Liu, Boqun Song, Wende Xiao, Haitao Zhou, Hongjun Gao in CAS, Min Ouyang in MU, and A.H. Castro Neto in SNU.) Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect.

  9. ARPES view on surface and bulk hybridization phenomena in the antiferromagnetic Kondo lattice CeRh2Si2.

    PubMed

    Patil, S; Generalov, A; Güttler, M; Kushwaha, P; Chikina, A; Kummer, K; Rödel, T C; Santander-Syro, A F; Caroca-Canales, N; Geibel, C; Danzenbächer, S; Kucherenko, Yu; Laubschat, C; Allen, J W; Vyalikh, D V

    2016-01-01

    The hybridization between localized 4f electrons and itinerant electrons in rare-earth-based materials gives rise to their exotic properties like valence fluctuations, Kondo behaviour, heavy-fermions, or unconventional superconductivity. Here we present an angle-resolved photoemission spectroscopy (ARPES) study of the Kondo lattice antiferromagnet CeRh2Si2, where the surface and bulk Ce-4f spectral responses were clearly resolved. The pronounced 4f (0) peak seen for the Ce terminated surface gets strongly suppressed in the bulk Ce-4f spectra taken from a Si-terminated crystal due to much larger f-d hybridization. Most interestingly, the bulk Ce-4f spectra reveal a fine structure near the Fermi edge reflecting the crystal electric field splitting of the bulk magnetic 4f (1)5/2 state. This structure presents a clear dispersion upon crossing valence states, providing direct evidence of f-d hybridization. Our findings give precise insight into f-d hybridization penomena and highlight their importance in the antiferromagnetic phases of Kondo lattices. PMID:26987899

  10. ARPES view on surface and bulk hybridization phenomena in the antiferromagnetic Kondo lattice CeRh2Si2

    PubMed Central

    Patil, S.; Generalov, A.; Güttler, M.; Kushwaha, P.; Chikina, A.; Kummer, K.; Rödel, T. C.; Santander-Syro, A. F.; Caroca-Canales, N.; Geibel, C.; Danzenbächer, S.; Kucherenko, Yu.; Laubschat, C.; Allen, J. W.; Vyalikh, D. V.

    2016-01-01

    The hybridization between localized 4f electrons and itinerant electrons in rare-earth-based materials gives rise to their exotic properties like valence fluctuations, Kondo behaviour, heavy-fermions, or unconventional superconductivity. Here we present an angle-resolved photoemission spectroscopy (ARPES) study of the Kondo lattice antiferromagnet CeRh2Si2, where the surface and bulk Ce-4f spectral responses were clearly resolved. The pronounced 4f 0 peak seen for the Ce terminated surface gets strongly suppressed in the bulk Ce-4f spectra taken from a Si-terminated crystal due to much larger f-d hybridization. Most interestingly, the bulk Ce-4f spectra reveal a fine structure near the Fermi edge reflecting the crystal electric field splitting of the bulk magnetic 4f 15/2 state. This structure presents a clear dispersion upon crossing valence states, providing direct evidence of f-d hybridization. Our findings give precise insight into f-d hybridization penomena and highlight their importance in the antiferromagnetic phases of Kondo lattices. PMID:26987899

  11. Delayed Methylene Blue Improves Lesion Volume, Multi-Parametric Quantitative Magnetic Resonance Imaging Measurements, and Behavioral Outcome after Traumatic Brain Injury.

    PubMed

    Talley Watts, Lora; Long, Justin Alexander; Boggs, Robert Cole; Manga, Hemanth; Huang, Shiliang; Shen, Qiang; Duong, Timothy Q

    2016-01-15

    Traumatic brain injury (TBI) remains a primary cause of death and disability in both civilian and military populations worldwide. There is a critical need for the development of neuroprotective agents that can circumvent damage and provide functional recovery. We previously showed that methylene blue (MB), a U.S. Food and Drug Administration-grandfathered drug with energy-enhancing and antioxidant properties, given 1 and 3 h post-TBI, had neuroprotective effects in rats. This study aimed to further investigate the neuroprotection of delayed MB treatment (24 h postinjury) post-TBI as measured by lesion volume and functional outcomes. Comparisons were made with vehicle and acute MB treatment. Multi-modal magnetic resonance imaging and behavioral studies were performed at 1 and 3 h and 2, 7, and 14 days after an impact to the primary forelimb somatosensory cortex. We found that delaying MB treatment 24 h postinjury still minimized lesion volume and functional deficits, compared to vehicle-treated animals. The data further support the potential for MB as a neuroprotective treatment, especially when medical teatment is not readily available. MB has an excellent safety profile and is clinically approved for other indications. MB clinical trials on TBI can thus be readily explored. PMID:25961471

  12. Delayed Methylene Blue Improves Lesion Volume, Multi-Parametric Quantitative Magnetic Resonance Imaging Measurements, and Behavioral Outcome after Traumatic Brain Injury.

    PubMed

    Talley Watts, Lora; Long, Justin Alexander; Boggs, Robert Cole; Manga, Hemanth; Huang, Shiliang; Shen, Qiang; Duong, Timothy Q

    2016-01-15

    Traumatic brain injury (TBI) remains a primary cause of death and disability in both civilian and military populations worldwide. There is a critical need for the development of neuroprotective agents that can circumvent damage and provide functional recovery. We previously showed that methylene blue (MB), a U.S. Food and Drug Administration-grandfathered drug with energy-enhancing and antioxidant properties, given 1 and 3 h post-TBI, had neuroprotective effects in rats. This study aimed to further investigate the neuroprotection of delayed MB treatment (24 h postinjury) post-TBI as measured by lesion volume and functional outcomes. Comparisons were made with vehicle and acute MB treatment. Multi-modal magnetic resonance imaging and behavioral studies were performed at 1 and 3 h and 2, 7, and 14 days after an impact to the primary forelimb somatosensory cortex. We found that delaying MB treatment 24 h postinjury still minimized lesion volume and functional deficits, compared to vehicle-treated animals. The data further support the potential for MB as a neuroprotective treatment, especially when medical teatment is not readily available. MB has an excellent safety profile and is clinically approved for other indications. MB clinical trials on TBI can thus be readily explored.

  13. Kondo effect at low electron density and high particle-hole asymmetry in 1D, 2D, and 3D

    NASA Astrophysics Data System (ADS)

    Žitko, Rok; Horvat, Alen

    2016-09-01

    Using the perturbative scaling equations and the numerical renormalization group, we study the characteristic energy scales in the Kondo impurity problem as a function of the exchange coupling constant J and the conduction-band electron density. We discuss the relation between the energy gain (impurity binding energy) Δ E and the Kondo temperature TK. We find that the two are proportional only for large values of J , whereas in the weak-coupling limit the energy gain is quadratic in J , while the Kondo temperature is exponentially small. The exact relation between the two quantities depends on the detailed form of the density of states of the band. In the limit of low electron density the Kondo screening is affected by the strong particle-hole asymmetry due to the presence of the band-edge van Hove singularities. We consider the cases of one- (1D), two- (2D), and three-dimensional (3D) tight-binding lattices (linear chain, square lattice, cubic lattice) with inverse-square-root, step-function, and square-root onsets of the density of states that are characteristic of the respective dimensionalities. We always find two different regimes depending on whether TK is higher or lower than μ , the chemical potential measured from the bottom of the band. For 2D and 3D, we find a sigmoidal crossover between the large-J and small-J asymptotics in Δ E and a clear separation between Δ E and TK for TK<μ . For 1D, there is, in addition, a sizable intermediate-J regime where the Kondo temperature is quadratic in J due to the diverging density of states at the band edge. Furthermore, we find that in 1D the particle-hole asymmetry leads to a large decrease of TK compared to the standard result obtained by approximating the density of states to be constant (flat-band approximation), while in 3D the opposite is the case; this is due to the nontrivial interplay of the exchange and potential scattering renormalization in the presence of particle-hole asymmetry. The 2D square

  14. Kondo Physics at Interfaces in Metallic Non-Local Spin Transport Devices

    NASA Astrophysics Data System (ADS)

    Leighton, Chris

    2015-03-01

    Despite the maturity of metallic spintronics there remain large gaps in our understanding of spin transport in metals, particularly with injection of spins across ferromagnetic/non-magnetic (FM/NM) interfaces, and their subsequent diffusion and relaxation. Unresolved issues include the limits of applicability of Elliott-Yafet spin relaxation, quantification of the influence of defects, surfaces, and interfaces on spin relaxation at nanoscopic dimensions, and the importance of magnetic and spin-orbit scattering. The non-local spin-valve is an enabling device in this context as, in addition to offering potentially disruptive applications, it allows for the separation of charge and spin currents. One particularly perplexing issue in metallic non-local spin valves is the widely observed non-monotonicity in the T-dependent spin accumulation, where the spin signal actually decreases at low T, in contrast to simple expectations. In this work, by studying an expanded range of FM/NM combinations (encompassing Ni80Fe20, Ni, Fe, Co, Cu, and Al), we demonstrate that this effect is not a property of a given FM or NM, but rather of the FM/NM pair. The non-monotonicity is in fact strongly correlated with the ability of the FM to form a dilute local magnetic moment in the NM. We show that local moments, resulting in this case from the ppm-level tail of the FM/NM interdiffusion profile, suppress the injected spin polarization and diffusion length via a novel manifestation of the Kondo effect, explaining all observations associated with the low T downturn in spin accumulation. We further show: (a) that this effect can be promoted by thermal annealing, at which point the conventional charge transport Kondo effect is simultaneously detected in the NM, and (b) that this suppression in spin accumulation can be quenched, even at interfaces that are highly susceptible to the effect, by insertion of a thin non-moment-supporting interlayer. Important implications for room temperature

  15. Substitutional effects on the electronic transport of the Kondo insulator Ce{sub 3}Bi{sub 4}Pt{sub 3}

    SciTech Connect

    Hundley, M.F.; Canfield, P.C.; Thompson, J.D.; Fisk, Z.

    1994-04-01

    The resistivity {rho} and thermoelectric power S of the doped Kondo insulator (Ce{sub 1-x}La{sub x}){sub 3}Bi{sub 4}Pt{sub 3} are examined to determine the effects of doping on the narrow gap exhibited by this compound. With increasing La concentration the energy gap progressively disappears in both {rho} and S and band-like transport develops below 25 K. The T-0 transport energy gap as determined from either {rho} or S scales with the single-impurity Kondo energy scale T{sub K} as determined from magnetic susceptibility measurements, independently of x for x {le} 0.25. This result strongly suggests that the gap arises from band hybridization that is driven by Kondo-like many-body correlations rather than from single-electronic interactions.

  16. Magnetic doping and kondo effect in bi(2)se(3) nanoribbons.

    PubMed

    Cha, Judy J; Williams, James R; Kong, Desheng; Meister, Stefan; Peng, Hailin; Bestwick, Andrew J; Gallagher, Patrick; Goldhaber-Gordon, David; Cui, Yi

    2010-03-10

    A simple surface band structure and a large bulk band gap have allowed Bi2Se3 to become a reference material for the newly discovered three-dimensional topological insulators, which exhibit topologically protected conducting surface states that reside inside the bulk band gap. Studying topological insulators such as Bi2Se3 in nanostructures is advantageous because of the high surface-to-volume ratio, which enhances effects from the surface states; recently reported Aharonov-Bohm oscillation in topological insulator nanoribbons by some of us is a good example. Theoretically, introducing magnetic impurities in topological insulators is predicted to open a small gap in the surface states by breaking time-reversal symmetry. Here, we present synthesis of magnetically doped Bi2Se3 nanoribbons by vapor-liquid-solid growth using magnetic metal thin films as catalysts. Although the doping concentration is less than approximately 2%, low-temperature transport measurements of the Fe-doped Bi2Se3 nanoribbon devices show a clear Kondo effect at temperatures below 30 K, confirming the presence of magnetic impurities in the Bi2Se3 nanoribbons. The capability to dope topological insulator nanostructures magnetically opens up exciting opportunities for spintronics.

  17. Tuning bulk and surface conduction in the proposed topological Kondo insulator SmB(6).

    PubMed

    Syers, Paul; Kim, Dohun; Fuhrer, Michael S; Paglione, Johnpierre

    2015-03-01

    Bulk and surface state contributions to the electrical resistance of single-crystal samples of the topological Kondo-insulator compound SmB_{6} are investigated as a function of crystal thickness and surface charge density, the latter tuned by ionic liquid gating with electrodes patterned in a Corbino disk geometry on a single (100) surface. By separately tuning bulk and surface conduction channels, we show conclusive evidence for a model with an insulating bulk and metallic surface states, with a crossover temperature that depends solely on the relative contributions of each conduction channel. The surface conductance, on the order of 100  e^{2}/h, exhibits a field-effect mobility of 133  cm^{2}/Vs and a large carrier density of ∼2×10^{14}  cm^{-2}, in good agreement with recent photoemission results. With the ability to gate modulate surface conduction by more than 25%, this approach provides promise for both fundamental and applied studies of gate-tuned devices structured on bulk crystal samples.

  18. Transport properties of the topological Kondo insulator SmB6 under the irradiation of light

    NASA Astrophysics Data System (ADS)

    Zhu, Guo-Bao; Yang, Hui-Min

    2016-10-01

    In this paper, we study transport properties of the X point in the Brillouin zone of the topological Kondo insulator SmB6 under the application of a circularly polarized light. The transport properties at high-frequency regime and low-frequency regime as a function of the ratio (κ) of the Dresselhaus-like and Rashba-like spin-orbit parameter are studied based on the Floquet theory and Boltzmann equation respectively. The sign of Hall conductivity at high-frequency regime can be reversed by the ratio κ and the amplitude of the light. The amplitude of the current can be enhanced by the ratio κ. Our findings provide a way to control the transport properties of the Dirac materials at low-frequency regime. Project supported by the National Natural Science Foundation of China (Grant Nos. 11504095 and 11447145), the Foundation of Heze University (Grant Nos. XY14B002 and XYPY01), and the Project funded by the Higher Educational Science and Technology Program of Shandong Province, China (Grant No. J15LJ55).

  19. Collective excitations from composite orders in Kondo lattice with non-Kramers doublets

    NASA Astrophysics Data System (ADS)

    Hoshino, S.; Kuramoto, Y.

    2015-03-01

    Goldstone modes emerge associated with spontaneous breakdown of the continuous symmetry in the two-channel Kondo lattice, which describes strongly correlated f-electron systems with a non-Kramers doublet at each site. This paper derives the spectra of these collective modes by the equation of motion method together with the random phase approximation. The diagonal composite order breaks the SU(2) channel symmetry, and the symmetry-restoring collective mode couples with magnetic field. On the other hand, the off-diagonal or superconducting composite order breaks the gauge symmetry of conduction electrons, and the collective mode couples with charge excitations near the zone boundary. At half-filling of the conduction bands, the spectra of these two modes become identical by a shift of the momentum, owing to the SO(5) symmetry of the system. The velocity of each Goldstone mode involves not only the Fermi velocity of conduction electrons but amplitude of the mean field as a multiplying factor. Detection of the Goldstone mode should provide a way to identify the composite order parameter.

  20. One-dimensional edge state transport in a topological Kondo insulator

    NASA Astrophysics Data System (ADS)

    Nakajima, Yasuyuki; Syers, Paul; Wang, Xiangfeng; Wang, Renxiong; Paglione, Johnpierre

    2016-03-01

    Topological insulators, with metallic boundary states protected against time-reversal-invariant perturbations, are a promising avenue for realizing exotic quantum states of matter, including various excitations of collective modes predicted in particle physics, such as Majorana fermions and axions. According to theoretical predictions, a topological insulating state can emerge from not only a weakly interacting system with strong spin-orbit coupling, but also in insulators driven by strong electron correlations. The Kondo insulator compound SmB6 is an ideal candidate for realizing this exotic state of matter, with hybridization between itinerant conduction electrons and localized f-electrons driving an insulating gap and metallic surface states at low temperatures. Here we exploit the existence of surface ferromagnetism in SmB6 to investigate the topological nature of metallic surface states by studying magnetotransport properties at very low temperatures. We find evidence of one-dimensional surface transport with a quantized conductance value of e2/h originating from the chiral edge channels of ferromagnetic domain walls, providing strong evidence that topologically non-trivial surface states exist in SmB6.

  1. Antiferromagnetic spin correlations and pseudogaplike behavior in Ca(Fe1-xCox)2As2 studied by 75As nuclear magnetic resonance and anisotropic resistivity

    DOE PAGES

    Cui, J.; Roy, B.; Tanatar, M. A.; Ran, S.; Bud'ko, S. L.; Prozorov, R.; Canfield, P. C.; Furukawa, Y.

    2015-11-06

    We report 75As nuclear magnetic resonance (NMR) measurements of single-crystalline Ca(Fe1–xCox)2As2 (x=0.023, 0.028, 0.033, and 0.059) annealed at 350°C for 7 days. From the observation of a characteristic shape of 75As NMR spectra in the stripe-type antiferromagnetic (AFM) state, as in the case of x=0 (TN=170 K), clear evidence for the commensurate AFM phase transition with the concomitant structural phase transition is observed in x=0.023 (TN=106 K) and x=0.028 (TN=53 K). Through the temperature dependence of the Knight shifts and the nuclear spin lattice relaxation rates (1/T1), although stripe-type AFM spin fluctuations are realized in the paramagnetic state as inmore » the case of other iron pnictide superconductors, we found a gradual decrease of the AFM spin fluctuations below a crossover temperature T* that was nearly independent of Co-substitution concentration, and it is attributed to a pseudogaplike behavior in the spin excitation spectra of these systems. The T* feature finds correlation with features in the temperature-dependent interplane resistivity, ρc(T), but not with the in-plane resistivity ρa(T). The temperature evolution of anisotropic stripe-type AFM spin fluctuations is tracked in the paramagnetic and pseudogap phases by the 1/T1 data measured under magnetic fields parallel and perpendicular to the c axis. As a result, based on our NMR data, we have added a pseudogaplike phase to the magnetic and electronic phase diagram of Ca(Fe1–xCox)2As2.« less

  2. Field dependence of the magnon dispersion in the Kondo lattice CeCu2 up to 12 T

    NASA Astrophysics Data System (ADS)

    Schedler, R.; Witte, U.; Rotter, M.; Loewenhaupt, M.; Schmidt, W.

    2005-05-01

    CeCu2 can be classified as a Kondo lattice which shows antiferromagnetic (AF) order below TN=3.5K [R. Trump et al., J. Appl. Phys. 69, 4699 (1991)]. The orthorhombic crystal and the simple AF magnetic structure with two magnetic moments in the primitive unit cell requires two magnon modes which are observed in zero and low magnetic fields and well described by spin wave theory. However, at higher fields, at and above 3T, an unexpected, additional magnetic excitation is observed. In contrast to the two low-energy magnon modes, it exhibits a steeper (factor 2) field dependence and a flat dispersion. Its origin is unclear.

  3. LABCOM resonator Phase 3

    SciTech Connect

    Keres, L.J.

    1990-11-01

    The purpose of this project was to develop quartz crystal resonator designs, production processes, and test capabilities for 5-MHz, 6.2-MHz, and 10-MHz resonators for Tactical Miniature Crystal Oscillator (TMXO) applications. GE Neutron Devices (GEND) established and demonstrated the capability to produce and test quartz crystal resonators for use in the TMXO developed by the US Army ERADCOM (now LABCOM). The goals in this project were based on the ERADCOM statement of work. The scope of work indicated that the resonator production facilities for this project would not be completely independent, but that they would be supported in part by equipment and processes in place at GEND used in US Department of Energy (DOE) work. In addition, provisions for production test equipment or or eventual technology transfer costs to a commercial supplier were clearly excluded from the scope of work. The demonstrated technical capability of the deep-etched blank design is feasible and practical. It can be manufactured in quantity with reasonable yield, and its performance is readily predictable. The ceramic flatpack is a very strong package with excellent hermeticity. The four-point mount supports the crystal to reasonable shock levels and does not perturb the resonator's natural frequency-temperature behavior. The package can be sealed with excellent yields. The high-temperature, high-vacuum processing developed for the TMXO resonator, including bonding the piezoid to its mount with conductive polyimide adhesive, is consistent with precision resonator fabrication. 1 fig., 6 tabs.

  4. Reprint of : Kondo effect in a carbon nanotube with spin-orbit interaction and valley mixing: A DM-NRG study

    NASA Astrophysics Data System (ADS)

    Mantelli, Davide; Paşcu Moca, Cătălin; Zaránd, Gergely; Grifoni, Milena

    2016-08-01

    We investigate the effects of spin-orbit interaction (SOI) and valley mixing on the transport and dynamical properties of a carbon nanotube (CNT) quantum dot in the Kondo regime. As these perturbations break the pseudo-spin symmetry in the CNT spectrum but preserve time-reversal symmetry, they induce a finite splitting Δ between formerly degenerate Kramers pairs. Correspondingly, a crossover from the SU(4) to the SU(2)-Kondo effect occurs as the strength of these symmetry breaking parameters is varied. Clear signatures of the crossover are discussed both at the level of the spectral function as well as of the conductance. In particular, we demonstrate numerically and support with scaling arguments that the Kondo temperature scales inversely with the splitting Δ in the crossover regime. In presence of a finite magnetic field, time reversal symmetry is also broken. We investigate the effects of both parallel and perpendicular fields (with respect to the tube's axis) and discuss the conditions under which Kondo revivals may be achieved.

  5. Closing the spin gap in the Kondo insulator Ce3Bi4Pt3 at high magnetic fields

    PubMed

    Jaime; Movshovich; Stewart; Beyermann; Berisso; Hundley; Canfield; Sarrao

    2000-05-11

    Kondo insulator materials--such as CeRhAs, CeRhSb, YbB12, Ce3Bi4Pt3 and SmB6--are 3d, 4f and 5f intermetallic compounds that have attracted considerable interest in recent years. At high temperatures, they behave like metals. But as temperature is reduced, an energy gap opens in the conduction band at the Fermi energy and the materials become insulating. This contrasts with other f-electron compounds, which are metallic at all temperatures. The formation of the gap in Kondo insulators has been proposed to be a consequence of hybridization between the conduction band and the f-electron levels, giving a 'spin' gap. If this is indeed the case, metallic behaviour should be recovered when the gap is closed by changing external parameters, such as magnetic field or pressure. Some experimental evidence suggests that the gap can be closed in SmB6 (refs 5, 8) and YbB12 (ref. 9). Here we present specific-heat measurements of Ce3Bi4Pt3 in d.c. and pulsed magnetic fields up to 60 tesla. Numerical results and the analysis of our data using the Coqblin-Schrieffer model demonstrate unambiguously a field-induced insulator-to-metal transition. PMID:10821266

  6. Light induced suppression of Kondo effect at amorphous LaAlO3/SrTiO3 interface

    NASA Astrophysics Data System (ADS)

    Liu, G. Z.; Qiu, J.; Jiang, Y. C.; Zhao, R.; Yao, J. L.; Zhao, M.; Feng, Y.; Gao, J.

    2016-07-01

    We report photoelectric properties of two-dimensional electron gas (2DEG) at an amorphous LaAlO3/SrTiO3 interface. Under visible light illumination (650 nm), an enhancement of electric conductivity is observed over the temperature range from 2 to 300 K. Particularly, a resistance upturn appearing below 25 K, which is further proved to from the Kondo effect, is suppressed by the 650 nm visible light. From the results of light-assisted Hall measurements, light irradiation increases the carrier mobility rather than carrier density in the Kondo regime. It is suggested that light induces the decoherence effect of localized spin states, hence the electron scattering is weakened and the carrier mobility is improved accordingly. Moreover, the enhancement of electrical conductivity by visible light verifies that in-gap states located in the SrTiO3 side of the interface play an important role in the electrical transport of the amorphous SrTiO3-based oxide 2DEG system. Our results provide deeper insight into the photoinduced effects in the 2DEG system, paving the way for the design of optoelectronic devices based on oxides.

  7. Competition between Kondo screening and Magnetism in the LaAlO3 /SrTiO3 Interface

    NASA Astrophysics Data System (ADS)

    Ruhman, Jonathan; Joshua, Arjun; Ilani, Shahal; Altman, Ehud

    2014-03-01

    We present a theory of magnetic phenomena at LaAlO3/SrTiO3 interfaces, which includes coupling between the conduction bands and local magnetic moments originating from charge traps at the interface. Tuning the itinerant electron density drives transitions between a heavy Fermi liquid phase with screened moments and various magnetic states. The dependence of the magnetic phenomena on the electron density stems from competing magnetic interactions between the local moments and the different conduction bands. At low densities only the lowest conduction band, composed of the dxy orbitals of Ti, is occupied. Its antiferromagnetic interaction with the local moments leads to screening of the moments at a Kondo scale that increases with density. However, above a critical density the dxz /dyz bands begin to populate. Their ferromagnetic interaction with the local moments competes with the antiferromagnetic interaction of the dxy band leading to eventual reduction of the Kondo scale with density. We explain the distinct magneto transport regimes seen in experiments as manifestations of the magnetic phase diagram computed from the model. We also present interpretation of previously unpublished data supporting the theoretical model.

  8. Competition between Kondo screening and magnetism at the LaAlO3/SrTiO3 interface

    NASA Astrophysics Data System (ADS)

    Ruhman, Jonathan; Joshua, Arjun; Ilani, Shahal; Altman, Ehud

    2014-09-01

    We present a theory of magnetic and magnetotransport phenomena at LaAlO3/SrTiO3 interfaces, which as a central ingredient includes coupling between the conduction bands and local magnetic moments originating from charge traps at the interface. Tuning the itinerant electron density in the model drives transitions between a heavy Fermi liquid phase with screened moments and various magnetic states. The dependence of the magnetic phenomena on the electron density or gate voltage stems from competing magnetic interactions between the local moments and the different conduction bands. At low densities only the lowest conduction band, composed of the dxy orbitals of Ti, is occupied. Its antiferromagnetic interaction with the local moments leads to screening of the moments at a Kondo scale that increases with density. However, above a critical density, measured in experiments to be nc≈1.7×1013cm-2, the dxz and dyz bands begin to populate. Their ferromagnetic interaction with the local moments competes with the antiferromagnetic interaction of the dxy band leading to eventual reduction of the Kondo scale with density. We explain the distinct magnetotransport regimes seen in experiments as manifestations of the magnetic phase diagram computed from the model. We present data showing a relation between the anomalous Hall effect and the resistivity in the system. The data strongly suggest that the concentration of local magnetic moments affecting the transport in the system is much lower than the carrier density, in accord with the theoretical model.

  9. Kondo versus indirect exchange: the role of the lattice and the actual range of RKKY interactions in real materials

    NASA Astrophysics Data System (ADS)

    Allerdt, Andrew; Feiguin, Adrian; Busser, Carlos; Martins, George

    2015-03-01

    Magnetic impurities embedded in a metal interact via an effective Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling mediated by the conduction electrons, which is commonly assumed to be long ranged, with an algebraic decay in the inter-impurity distance. However, they can also form a Kondo screened state that is oblivious to the presence of other impurities. We study the competition mechanisms between both effects on the square and cubic lattices by introducing an exact mapping onto an effective one-dimensional problem that we can solve with the density matrix renormalization group method (DMRG). We show a dramatic departure from the conventional RKKY theory, that can be attributed to the dimensionality and different densities of states, as well as the quantum nature of the magnetic moments. In particular, for dimension d > 1 , Kondo physics dominates even at short distances, while the ferromagnetic RKKY state is energetically unfavorable. Our findings can have clear implications in the interpretation of experiments and for tailoring the magnetic properties of surfaces.

  10. Competition between Kondo and indirect exchange at the edges and bulk of graphene, and 2D materials

    NASA Astrophysics Data System (ADS)

    Allerdt, Andrew; Martins, George; Feiguin, Adrian

    We study the problem of two magnetic impurities at the surface of graphene, BN, MoS2, phosphorene, silicene and germanene using exact numerical methods. We map the band structure of these materials onto one dimensional tight-binding chains in the same spirit as Wilson's numerical renormalization group. We use the density matrix renormalization group to solve the problem exactly, keeping all the information about the underlying lattice. Competition between Kondo and Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions is non-trivial, due to strong non-perturbative effects. Depending on the presence of a pseudogap, or gap, we identify an important directionality and position dependence of the correlations. We present scenarios and regimes where impurities prefer to form their own Kondo clouds instead of an RKKY singlet state, or remain as uncoupled local moments. In the particular case of graphene, ferromagnetism is only stable at half-filling. In addition, we study the effects of spin-orbit coupling, and the presence of edge states.

  11. Ultrafast terahertz spectroscopy study of Kondo insulating thin film SmB6: evidence for an emergent surface state

    NASA Astrophysics Data System (ADS)

    Zhang, Jingdi; Yong, Jie; Takeuchi, Ichiro; Greene, Richard; Averitt, Richard

    We utilize terahertz time domain spectroscopy to investigate thin films of the heavy fermion compound SmB6, a prototype Kondo insulator. Temperature dependent terahertz (THz) conductivity measurements reveal a rapid decrease in the Drude weight and carrier scattering rate at ~T* =20 K, well below the hybridization gap onset temperature (100 K). Moreover, a low-temperature conductivity plateau (below 20K) indicates the emergence of a surface state with an effective electron mass of 0.1me. Conductivity dynamics following optical excitation are also measured and interpreted using Rothwarf-Taylor (R-T) phenomenology, yielding a hybridization gap energy of 17 meV. However, R-T modeling of the conductivity dynamics reveals a deviation from the expected thermally excited quasiparticle density at temperatures below 20K, indicative of another channel opening up in the low energy electrodynamics. Taken together, these results suggest the onset of a surface state well below the crossover temperature (100K) after long-range coherence of the f-electron Kondo lattice is established. JZ and RDA acknowledge support from DOE - Basic Energy Sciences under Grant No. DE-FG02-09ER46643, under which the THz measurements and data analysis were performed. JY, IT and RLG acknowledge support from ONR N00014-13-1-0635 and NSF DMR 1410665.

  12. Optical resonator

    NASA Technical Reports Server (NTRS)

    Taghavi-Larigani, Shervin (Inventor); Vanzyl, Jakob J. (Inventor); Yariv, Amnon (Inventor)

    2006-01-01

    The invention discloses a semi-ring Fabry-Perot (SRFP) optical resonator structure comprising a medium including an edge forming a reflective facet and a waveguide within the medium, the waveguide having opposing ends formed by the reflective facet. The performance of the SRFP resonator can be further enhanced by including a Mach-Zehnder interferometer in the waveguide on one side of the gain medium. The optical resonator can be employed in a variety of optical devices. Laser structures using at least one SRFP resonator are disclosed where the resonators are disposed on opposite sides of a gain medium. Other laser structures employing one or more resonators on one side of a gain region are also disclosed.

  13. Fano resonances in magnetic metamaterials

    SciTech Connect

    Naether, Uta; Molina, Mario I.

    2011-10-15

    We study the scattering of magnetoinductive plane waves by internal (external) capacitive (inductive) defects coupled to a one-dimensional split-ring resonator array. We examine a number of simple defect configurations where Fano resonances occur and study the behavior of the transmission coefficient as a function of the controllable external parameters. We find that for embedded capacitive defects, the addition of a small amount of coupling to second neighbors is necessary for the occurrence of Fano resonance. For external inductive defects, Fano resonances are commonplace, and they can be tuned by changing the relative orientation or distance between the defect and the SSR array.

  14. Hydro-acoustic resonance behavior in presence of a precessing vortex rope: observation of a lock-in phenomenon at part load Francis turbine operation

    NASA Astrophysics Data System (ADS)

    Favrel, A.; Landry, C.; Müller, A.; Yamamoto, K.; Avellan, F.

    2014-03-01

    Francis turbines operating at part load condition experience the development of a cavitating helical vortex rope in the draft tube cone at the runner outlet. The precession movement of this vortex rope induces local convective pressure fluctuations and a synchronous pressure pulsation acting as a forced excitation for the hydraulic system, propagating in the entire system. In the draft tube, synchronous pressure fluctuations with a frequency different to the precession frequency may also be observed in presence of cavitation. In the case of a matching between the precession frequency and the synchronous surge frequency, hydro-acoustic resonance occurs in the draft tube inducing high pressure fluctuations throughout the entire hydraulic system, causing torque and power pulsations. The risk of such resonances limits the possible extension of the Francis turbine operating range. A more precise knowledge of the phenomenon occurring at such resonance conditions and prediction capabilities of the induced pressure pulsations needs therefore to be developed. This paper proposes a detailed study of the occurrence of hydro-acoustic resonance for one particular part load operating point featuring a well-developed precessing vortex rope and corresponding to 64% of the BEP. It focuses particularly on the evolution of the local interaction between the pressure fluctuations at the precession frequency and the synchronous surge mode passing through the resonance condition. For this purpose, an experimental investigation is performed on a reduced scale model of a Francis turbine, including pressure fluctuation measurements in the draft tube and in the upstream piping system. Changing the pressure level in the draft tube, resonance occurrences are highlighted for different Froude numbers. The evolution of the hydro-acoustic response of the system suggests that a lock-in effect between the excitation frequency and the natural frequency may occur at low Froude number, inducing a hydro

  15. Scaling behavior of temperature-dependent thermopower in CeAu2Si2 under pressure

    NASA Astrophysics Data System (ADS)

    Ren, Z.; Scheerer, G. W.; Lapertot, G.; Jaccard, D.

    2016-07-01

    We report a combined study of in-plane resistivity and thermopower of the pressure-induced heavy-fermion superconductor CeAu2Si2 up to 27.8 GPa. It is found that thermopower follows a scaling behavior in T /T* almost up to the magnetic critical pressure pc˜22 GPa. By comparing with resistivity results, we show that the magnitude and characteristic temperature dependence of thermopower in this pressure range are governed by the Kondo coupling and crystal-field splitting, respectively. Below pc, the superconducting transition is preceded by a large negative thermopower minimum, suggesting a close relationship between the two phenomena. Furthermore, thermopower of a variety of Ce-based Kondo lattices with different crystal structures follows the same scaling relation up to T /T*˜2 .

  16. Resonance vibrations of buried landmines

    NASA Astrophysics Data System (ADS)

    Zagrai, Andrei N.; Donskoy, Dimitri M.; Ekimov, Alexander E.

    2004-09-01

    Resonance behavior of many types of landmines was first experimentally discovered in 2000 (Donskoy et al. in Proceedings of SPIE Vol. 4394, pp. 575-582, 2001). Laboratory studies and field tests have shown that mine"s resonance response is a complex phenomenon dependent upon interaction between soil and mines and their respective properties. Although the resonance effect was successfully used by various research teams for detection of landmines, there were no thorough studies on various factors influencing buried mine's resonance response. This paper presents results of theoretical and experimental investigation of this problem including multi-modal structure of mine's vibration response, effect of burial depth and soil condition. In the modeling efforts we considered multiple modes of vibration of mine casing and represented them as oscillators with effective parameters. This approach allowed for simplification of analysis and expanding existing lump-element model to account for multiple vibration modes. The experimental tests were focused on studying the effects of burial depth and soil moisture content on resonance behavior of soil-mine system. The tests have shown that a resonance frequency initially decreases with burial depth, as expected. However, an anomalous resonance frequency increase was observed at greater depths; soil moisture even further increases the resonance frequency.

  17. Shape resonances in molecular fields

    SciTech Connect

    Dehmer, Joseph L.

    1984-01-01

    A shape resonance is a quasibound state in which a particle is temporarily trapped by a potential barrier (i.e., the shape of the potential), through which it may eventually tunnel and escape. This simple mechanism plays a prominent role in a variety of excitation processes in molecules, ranging from vibrational excitation by slow electrons to ionization of deep core levels by x-rays. Moreover, their localized nature makes shape resonances a unifying link between otherwise dissimilar circumstances. One example is the close connection between shape resonances in electron-molecule scattering and in molecular photoionization. Another is the frequent persistence of free-molecule shape resonant behavior upon adsorption on a surface or condensation into a molecular solid. The main focus of this article is a discussion of the basic properties of shape resonances in molecular fields, illustrated by the more transparent examples studied over the last ten years. Other aspects to be discussed are vibrational effects of shape resonances, connections between shape resonances in different physical settings, and examples of shape resonant behavior in more complex cases, which form current challenges in this field.

  18. Tuning the ground state of the Kondo lattice in UT Bi2 (T = Ag, Au) single crystals

    NASA Astrophysics Data System (ADS)

    Rosa, Priscila; Luo, Yongkang; Pagliuso, Pascoal; Bauer, Eric; Thompson, Joe; Fisk, Zachary

    2015-03-01

    Motivated by the interesting magnetic anisotropy found in the Ce-based heavy fermion family Ce TX2 (T = transition metal, X = pnictogen), here we study the novel U-based parent compounds U TBi2 (T = Ag, Au) by combining magnetization, electrical resistivity, and heat-capacity measurements. The single crystals, synthesized by the self-flux method, also crystallize in the tetragonal HfCuSi2-type structure (space group P4/nmm). Interestingly, although UAgBi2 is a low- γ antiferromagnet below TN = 181 K, UAuBi2 is a moderately heavy uniaxial ferromagnet below Tc = 22 K. Nevertheless, both compounds display the easy-magnetization direction along the c-axis and a large magnetocrystalline anisotropy. Our results point out to an incoherent Kondo behaviour in the paramagnetic state and an intricate competition between crystal field effects and two anisotropic exchange interactions, which lead to the remarkable difference in the observed ground states.

  19. Heavy surface state in a possible topological Kondo insulator: Magnetothermoelectric transport on the (011) plane of SmB6

    DOE PAGES

    Luo, Yongkang; Chen, Hua; Dai, Jianhui; Xu, Zhu -an; Thompson, J. D.

    2015-02-25

    Motivated by the high sensitivity to Fermi surface topology and scattering mechanisms in magnetothermoelectric transport, we have measured the thermopower and Nernst effect on the (011) plane of the proposed topological Kondo insulator SmB6. These experiments, together with electrical resistivity and Hall effect measurements, suggest that the (011) plane also harbors a metallic surface with an effective mass on the order of 10–102 m0. The surface and bulk conductances are well distinguished in these measurements and are categorized into metallic and nondegenerate semiconducting regimes, respectively. As a result, electronic correlations play an important role in enhancing scattering and also contributemore » to the heavy surface state.« less

  20. Julius Edgar Lilienfeld Prize: Lilienfeld Prize Lecture: Emergent Behavior in Quantum Matter

    NASA Astrophysics Data System (ADS)

    Pines, David

    We live in an emergent universe in which interactions between the basic building blocks of matter and their environment give rise to unpredicted and unexpected emergent behavior at every scale. As physicists we seek to identify the organizing principles responsible for that behavior, construct soluble models that incorporate these, and explain experiment. In this lecture, I illustrate this approach to understanding emergent behavior in quantum matter through three examples: collective modes in electron, helium, and nuclear liquids; the emergence of superconductivity in conventional and unconventional superconductors, nuclei, and neutron stars; and the emergence of heavy electrons in Kondo lattice materials.

  1. Crystal-field states of Kondo lattice heavy fermions CeRuSn3 and CeRhSn3

    NASA Astrophysics Data System (ADS)

    Anand, V. K.; Adroja, D. T.; Britz, D.; Strydom, A. M.; Taylor, J. W.; Kockelmann, W.

    2016-07-01

    Inelastic neutron scattering experiments have been carried out to determine the crystal-field states of the Kondo lattice heavy fermions CeRuSn3 and CeRhSn3. Both the compounds crystallize in LaRuSn3-type cubic structure (space group P m 3 ¯n ) in which the Ce atoms occupy two distinct crystallographic sites with cubic (m 3 ¯ ) and tetragonal (4 ¯m .2 ) point symmetries. The INS data of CeRuSn3 reveal the presence of a broad excitation centered around 6-8 meV, which is accounted by a model based on crystal electric field (CEF) excitations. On the other hand, the INS data of isostructural CeRhSn3 reveal three CEF excitations around 7.0, 12.2, and 37.2 meV. The neutron intensity sum rule indicates that the Ce ions at both cubic and tetragonal Ce sites are in Ce3 + state in both CeRuSn3 and CeRhSn3. The CEF level schemes for both the compounds are deduced. We estimate the Kondo temperature TK=3.1 (2 ) K for CeRuSn3 from neutron quasielastic linewidth in excellent agreement with that determined from the scaling of magnetoresistance which gives TK=3.2 (1 ) K. For CeRhSn3, the neutron quasielastic linewidth gives TK≈4.6 K. For both CeRuSn3 and CeRhSn3, the ground state of Ce3 + turns out to be a quartet for the cubic site and a doublet for the tetragonal site.

  2. Evolution from a non-Fermi liquid Kondo lattice to intermediate valence behaviour in CeRhSn(1-x)In(x).

    PubMed

    Ślebarski, A; Fijałkowski, M; Goraus, J

    2012-03-28

    We present investigations of the magnetic and electric transport properties, specific heat, and electronic structure of the intermetallic and strongly correlated system of CeRhSn(1-x)In(x) compounds. The main goal of this paper is to determine the hybridization energy between the f electron and conduction electron states, V(cf), and its influence on the ground state properties of the system. The complementary experimental data are discussed on the basis of the Anderson model for a periodic Kondo lattice. CeRhSn is known as a non-Fermi liquid, while CeRhIn is a valence fluctuating system. We discuss the ground state properties of CeRhSn(1-x)In(x) and compare the results with those obtained for the doped Ce-based Kondo insulators.

  3. Evolution from a non-Fermi liquid Kondo lattice to intermediate valence behaviour in CeRhSn(1-x)In(x).

    PubMed

    Ślebarski, A; Fijałkowski, M; Goraus, J

    2012-03-28

    We present investigations of the magnetic and electric transport properties, specific heat, and electronic structure of the intermetallic and strongly correlated system of CeRhSn(1-x)In(x) compounds. The main goal of this paper is to determine the hybridization energy between the f electron and conduction electron states, V(cf), and its influence on the ground state properties of the system. The complementary experimental data are discussed on the basis of the Anderson model for a periodic Kondo lattice. CeRhSn is known as a non-Fermi liquid, while CeRhIn is a valence fluctuating system. We discuss the ground state properties of CeRhSn(1-x)In(x) and compare the results with those obtained for the doped Ce-based Kondo insulators. PMID:22369764

  4. Upper critical field and Kondo effects in Fe(Te0.9Se0.1) thin films by pulsed field measurements

    DOE PAGES

    Salamon, Myron B.; Cornell, Nicholas; Jaime, Marcelo; Balakirev, Fedor F.; Zakhidov, Anvar; Huang, Jijie; Wang, Haiyan

    2016-02-10

    The transition temperatures of epitaxial films of Fe(Te0:9Se0:1) are remarkably insensitive to applied magnetic field, leading to predictions of upper critical fields Bc2(T = 0) in excess of 100 T. Using pulsed magnetic fields, we find Bc2(0) to be on the order of 45 T, similar to values in bulk material and still in excess of the paramagnetic limit. The same films show strong magnetoresistance in fields above Bc2(T), consistent with the observed Kondo minimum seen above Tc. Fits to the temperature dependence in the context of the WHH model, using the experimental value of the Maki parameter, require anmore » effective spin-orbit relaxation parameter of order unity. Lastly, we suggest that Kondo localization plays a similar role to spin-orbit pair breaking in making WHH fits to the data.« less

  5. Strongly-disordered hybridization and non-Fermi liquid behavior in CePt4Ge12-xSbx studied with thermoelectric power

    NASA Astrophysics Data System (ADS)

    White, Benjamin; Huang, Kevin; Maple, M. Brian

    2014-03-01

    Non-Fermi liquid (NFL) behavior is commonly associated with the presence of a nearby quantum critical point, but can also be observed in other scenarios. In a clean system, hybridization between localized and itinerant electron states can be characterized by a single Kondo temperature TK, but introducing chemical disorder can lead to a wide distribution of TK values. Given sufficient disorder, the resulting distribution will tend to include an appreciable number of localized electron states which are characterized by TK ~ 0 K, and NFL behavior emerges. A Kondo-disorder type of NFL behavior was recently reported in the filled skutterudite system CePt4Ge12-xSbx in the vicinity of x = 1 . We performed a study of the thermoelectric power S(T) for this system and observed an evolution of S(T) with x that is dramatic and broadly consistent with the boundaries of the proposed phase diagram. The effect of disordered hybridization is clearly observed in a low-temperature feature in S(T) in the range 0 . 5 <= x <= 1 . 5 and NFL behavior is also observed at x = 1. These results clearly demonstrate how sensitively S(T) is able to probe a Kondo disorder system. Research was performed with support from the US DOE grant DE-FG02-04-ER46105.

  6. Kondo screening and spin excitation in few-layer CoPc molecular assembly stacking on Pb(111) surface: A DFT+HEOM study

    NASA Astrophysics Data System (ADS)

    Wang, Yu; Zheng, Xiao; Yang, Jinlong

    2016-10-01

    Transition metal phthalocyanine molecules adsorbed on a metal substrate exhibit rich spin-related phenomena such as magnetic anisotropy, spin excitation, and Kondo effect. In this work, we investigate theoretically few-layer cobalt phthalocyanine (CoPc) molecular assembly stacking on Pb(111) surface with the use of a combined density functional theory (DFT) and hierarchical equations of motion (HEOM) approach. Calculation results indicate that the local spin properties of CoPc/Pb(111) composites depend critically on the number of adsorption layers. The first layer of CoPc on the Pb(111) surface serves as a spin-insulating buffer, while the CoPc molecules in the second layer exhibit spin-1/2 Kondo effect with a Kondo temperature of about 22 K. In a triple-layer CoPc assembly stacking on Pb(111), the antiferromagnetic coupling between the second and third layers leads to local spin-flip excitations under finite bias voltages, which gives rise to characteristic signatures in the differential conductance spectra. The DFT+HEOM approach thus provides a practical means for investigating the local electronic and spin properties of two-dimensional molecular assemblies adsorbed on the metal surface. The insights obtained from the first-principles based simulations could be useful for experimental manipulation or design of magnetic composite systems.

  7. Effect of calcium on structure and function of a hyaluronic acid matrix: Carbon-13 nuclear magnetic resonance analysis and the diffusional behavior of small solutes

    PubMed Central

    Napier, Mary A.; Hadler, Nortin M.

    1978-01-01

    Natural-abundance 13C NMR at 25.16 MHz has been used to study a 2.5% matrix of hyaluronic acid at various degrees of polymerization and at various ionic strengths. Peak assignment is facilitated by comparing proton-decoupled and off-resonance-decoupled spectra of a hyaluronidase-depolymerized matrix with spectra from relevant monosaccharides. In contrast to the spectrum following depolymerization, the spectrum for intact matrix has considerable broadening, particularly for peaks assigned to the N-acetylglucosamine moiety. This is most dramatic for the hydroxymethylene carbon. With the addition of Ca2+ above 5 mM these broadened peaks narrow and approach the sharpness observed for the hyaluronidase digest. There is no shift in resonance peak positions. These changes are quantitatively less impressive if Na+ is substituted for Ca2+. The data suggest the existence of a considerable degree of order in regions of the matrix at physiological concentrations of Ca2+. Within such a matrix the translational movement of lysine and glucose is enhanced relative to that in a matrix of agarose. Further addition of Ca2+ abrogates not only matrix order, but the enhanced diffusivity as well. PMID:276867

  8. Triacontanol and jasmonic acid differentially modulate the lipid organization as evidenced by the fluorescent probe behavior and 31P nuclear magnetic resonance shifts in model membranes.

    PubMed

    Sivakumar Swamy, G; Swamy, Sivakumar G; Ramanarayan, K; Inamdar, Laxmi S; Inamdar, Sanjeev R

    2009-04-01

    Fluorescence resonance energy transfer (FRET), time-resolved fluorescence and anisotropy decays were determined in large unilamellar vesicles (LUVs) of egg phosphatidylcholine with the FRET pair N-(7-nitrobenz-2-oxa-1,3-diazol-4-yl)-1,2-dipalmitoyl-sn-glycero-3-phospho-ethanolamine as donor and lissamine rhodamine B 1,2-dipalmitoyl-sn-glycero-3-phosphoethanolamine as acceptor, using 2-ps pulses from a Ti:sapphire laser on LUVs with incorporated plant growth regulators: triacontanol (TRIA) and jasmonic acid (JA). FRET efficiency, energy transfer rate, rotation correlation time, microviscosity, and diffusion coefficient of lateral diffusion of lipids were calculated from these results. It was observed that TRIA and JA differentially modulated all parameters studied. The effect of JA in such modulations was always partially reversed by TRIA. Also, the generalized polarization of laurdan fluorescence indicated that JA enhances the degree of hydration in lipid bilayers to a larger extent than does TRIA. Solid-state (31)P magic-angle spinning nuclear magnetic resonance spectra of LUVs showed two chemical shifts, at 0.009 and -11.988 ppm, at low temperatures (20 degrees C), while at increasing temperatures (20-60 degrees C) only one (at -11.988 ppm) was prominent and the other (0.009 ppm) gradually became obscure. However, LUVs with TRIA exhibited only one of the shifts at 0.353 ppm even at lower temperatures and JA did not affect the chemical shifts.

  9. The Kondo problem. II. Crossover from asymptotic freedom to infrared slavery

    NASA Astrophysics Data System (ADS)

    Schlottmann, P.

    1982-04-01

    In the preceding paper we transformed the s-d Hamiltonian onto a resonance level with a large perturbation and derived the scaling equations for the vertices, the invariant coupling, and the resonance width. The scaling equations are integrated under the assumption that the energy dependence of the resonance width can be neglected. The transcendental equation obtained in this way for the renormalized resonance width is solved in the relevant limits and allows a calculation of the static and dynamical susceptibility. At high temperatures the perturbation expansion for the relaxation rate and the susceptibility is reproduced up to third order in Jρ. At low temperatures the lifetime and χ0 remain finite and vary according to a Fermi-liquid theory. The approximation scheme interpolates in this way between the asymptotic freedom and the infrared slavery, yielding a smooth crossover. The present results are in quantitative agreement with previous ones obtained with the relaxation-kernel method by Götze and Schlottmann. The advantages and drawbacks of the method are discussed. The calculation of the dynamical susceptibility is extended to nonzero external magnetic fields. The quasielastic peak of χ''(ω)ω is suppressed at low temperatures and large magnetic fields and shoulders develop at ω=+/-B.

  10. Influence of the colloidal structure of dairy gels on milk fat fusion behavior: quantification of the liquid fat content by in situ quantitative proton nuclear magnetic resonance spectroscopy (isq (1) H NMR).

    PubMed

    Bouteille, Romain; Perez, Jeanne; Khifer, Farid; Jouan-Rimbaud-Bouveresse, Delphine; Lecanu, Bruno; This, Hervé

    2013-04-01

    Dairy gels (DG), such as yoghurts, contain both solid and liquid fats at the time of consumption, as their temperature rises to anything between 10 and 24 °C after being introduced into the mouth at 4 °C. The mass ratio between solid and liquid fats, which depends on the temperature, impacts the organoleptic properties of DG. As the ordinary methods for determining this ratio can only be applied to samples consisting mainly in fat materials, a fat extraction step needs to be added into the analytical process when applied to DG, which prevents the study of the potential impact of their colloidal structure on milk fat fusion behavior. In situ quantitative proton nuclear magnetic resonance spectroscopy (isq (1) H NMR) was investigated as a method for direct measurements in DG: at temperatures between 20.0 and 70.0 °C, the liquid fat content and the composition of triacylglycerols of the liquid phase (in terms of alkyl chains length) were determined. Spectra of isolated milk fat also enable the quantification of the double bonds of triacylglycerols. Statistical tests showed no significant difference between isolated milk fat and milk fat inside a DG in terms of melting behavior: the fat globule membrane does not seem to have a significant influence on the fat melting behavior.

  11. Influence of the colloidal structure of dairy gels on milk fat fusion behavior: quantification of the liquid fat content by in situ quantitative proton nuclear magnetic resonance spectroscopy (isq (1) H NMR).

    PubMed

    Bouteille, Romain; Perez, Jeanne; Khifer, Farid; Jouan-Rimbaud-Bouveresse, Delphine; Lecanu, Bruno; This, Hervé

    2013-04-01

    Dairy gels (DG), such as yoghurts, contain both solid and liquid fats at the time of consumption, as their temperature rises to anything between 10 and 24 °C after being introduced into the mouth at 4 °C. The mass ratio between solid and liquid fats, which depends on the temperature, impacts the organoleptic properties of DG. As the ordinary methods for determining this ratio can only be applied to samples consisting mainly in fat materials, a fat extraction step needs to be added into the analytical process when applied to DG, which prevents the study of the potential impact of their colloidal structure on milk fat fusion behavior. In situ quantitative proton nuclear magnetic resonance spectroscopy (isq (1) H NMR) was investigated as a method for direct measurements in DG: at temperatures between 20.0 and 70.0 °C, the liquid fat content and the composition of triacylglycerols of the liquid phase (in terms of alkyl chains length) were determined. Spectra of isolated milk fat also enable the quantification of the double bonds of triacylglycerols. Statistical tests showed no significant difference between isolated milk fat and milk fat inside a DG in terms of melting behavior: the fat globule membrane does not seem to have a significant influence on the fat melting behavior. PMID:23464867

  12. Laser Resonator

    NASA Technical Reports Server (NTRS)

    Harper, L. L. (Inventor)

    1983-01-01

    An optical resonator cavity configuration has a unitary mirror with oppositely directed convex and concave reflective surfaces disposed into one fold and concertedly reversing both ends of a beam propagating from a laser rod disposed between two total internal reflection prisms. The optical components are rigidly positioned with perpendicularly crossed virtual rooflines by a compact optical bed. The rooflines of the internal reflection prisms, are arranged perpendicularly to the axis of the laser beam and to the optical axes of the optical resonator components.

  13. Resonance conditions

    NASA Astrophysics Data System (ADS)

    Rebusco, P.

    2005-11-01

    Non-linear parametric resonances occur frequently in nature. Here we summarize how they can be studied by means of perturbative methods. We show in particular how resonances can affect the motion of a test particle orbiting in the vicinity of a compact object. These mathematical toy-models find application in explaining the structure of the observed kHz Quasi-Periodic Oscillations: we show which aspects of the reality naturally enter in the theory, and which one still remain a puzzle.

  14. Autostereogram resonators

    NASA Astrophysics Data System (ADS)

    Leavey, Sean; Rae, Katherine; Murray, Adam; Courtial, Johannes

    2012-09-01

    Autostereograms, or "Magic Eye" pictures, are repeating patterns designed to give the illusion of depth. Here we discuss optical resonators that create light patterns which, when viewed from a suitable position by a monocular observer, are autostereograms of the three-dimensional shape of one of the mirror surfaces.

  15. Ferromagnetic critical behavior in U(Co1-xFex)Al (0 ≤x ≤0.02 ) studied by 59Co nuclear quadrupole resonance measurements

    NASA Astrophysics Data System (ADS)

    Karube, K.; Hattori, T.; Ishida, K.; Kimura, N.

    2015-02-01

    In order to investigate physical properties around a ferromagnetic (FM) quantum transition point and a tricritical point (TCP) in the itinerant-electron metamagnetic compound UCoAl, we have performed the 59Co nuclear quadrupole resonance (NQR) measurement for the Fe-substituted U(Co1-xFex)Al(x =0 ,0.5 ,1 ,and2 %) in zero external magnetic field. The Fe concentration dependence of 59Co -NQR spectra at low temperatures indicates that the first-order FM transition occurs at least above x =1 % . The magnetic fluctuations along the c axis detected by the nuclear spin-spin relaxation rate 1 /T2 exhibit an anomaly at Tmax˜20 K and enhance with increasing x . These results are in good agreement with theoretical predictions and indicate the presence of prominent critical fluctuations at the TCP in this system.

  16. Theoretical and experimental investigation of microstrip rhombic resonators

    NASA Astrophysics Data System (ADS)

    Al-Charchafchi, S. H.; Boulkos, J.

    1990-06-01

    The resonant behavior of a novel microstrip rhombic resonator is investigated by analyzing an equivalent circuit based on transmission line modeling. Design curves showing the dependence of resonator performance on its parameters, as well as the substrate parameters, are presented. Experiments carried out showed a significant reduction in insertion loss when the rhombic resonator is dielectrically shielded. The resonator could be used as a microwave bandpass filter or a stabilization circuit for microwave oscillators in both hybrid and monolithic integrated circuits.

  17. Apparatus for investigating resonance with application to magnetic resonance imaging

    NASA Astrophysics Data System (ADS)

    Murphy, Sytil; Jones, Dyan L.; Gross, Josh; Zollman, Dean

    2015-11-01

    Resonance is typically studied in the context of either a pendulum or a mass on a spring. We have developed an apparatus that enables beginning students to investigate resonant behavior of changing magnetic fields, in addition to the properties of the magnetic field due to a wire and the superposition of magnetic fields. In this resonant system, a compass oscillates at a frequency determined by the compass's physical properties and an external magnetic field. While the analysis is mathematically similar to that of the pendulum, this apparatus has an advantage that the magnetic field is easily controlled, while it is difficult to control the strength of gravity. This apparatus has been incorporated into a teaching module on magnetic resonance imaging.

  18. Tunable Dirac-point resonance induced by a STM-coupled Anderson impurity on a topological insulator surface

    NASA Astrophysics Data System (ADS)

    Deng, Ming-Xun; Wang, Rui-Qiang; Luo, Wei; Sheng, L.; Wang, B. G.; Xing, D. Y.

    2016-09-01

    The interaction effect between the surface states of a topological insulator (TI) and a STM-coupled Anderson impurity is studied by using equations of motion of the Green’s functions. Remarkably, we show that when a coupling between the Anderson impurity and the STM tip is included, the tunneling resonance and the Kondo peak can be tuned to be exactly at the Dirac point, by adjusting the impurity level and Fermi energy, such that the local density of states at the Dirac point is significantly enhanced. This is in contrast to the case of a STM-decoupled Anderson impurity, where both resonances are always fully suppressed at the Dirac point. Our finding suggests a pathway to experimentally control the fundamental properties of the electrons on a TI surface.

  19. Light-dependent and -independent behavioral effects of extremely low frequency magnetic fields in a land snail are consistent with a parametric resonance mechanism

    SciTech Connect

    Prato, F.S.; Thomas, A.W. |; Kavaliers, M.; Cullen, A.P.

    1997-05-01

    Exposure to extremely low frequency (ELF) magnetic fields has been shown to attenuate endogenous opioid peptide mediated antinociception or analgesia in the terrestrial pulmonate snail, Cepaea nemoralis. Here the authors examine the roles of light in determining this effect and address the mechanisms associated with mediating the effects of the ELF magnetic fields in both the presence and absence of light. Specifically, they consider whether the magnetic field effects involve an indirect induced electric current mechanism or a direct effect such as a parametric resonance mechanism (PRM). They exposed snails in both the presence and absence of light at three different frequencies (30, 60, and 120 Hz) with static field values (B{sub DC}) and ELF magnetic field amplitude (peak) and direction (B{sub AC}) set according to the predictions of the PRM for Ca{sup 2+}. Analgesia was induced in snails by injecting them with an enkephalinase inhibitor, which augments endogenous opioid (enkephalin) activity. They found that the magnetic field exposure reduced this opioid-induced analgesia significantly more if the exposure occurred in the presence rather than the absence of light. However, the percentage reduction in analgesia in both the presence and absence of light was not dependent on the ELF frequency. This finding suggests that in both the presence and the absence of light the effect of the ELF magnetic field was mediated by a direct magnetic field detection mechanism such as the PRM rather than an induced current mechanism.

  20. Sandwich-like Cu1.94S-ZnS-Cu1.94S nanoheterostructure: structure, formation mechanism and localized surface plasmon resonance behavior

    NASA Astrophysics Data System (ADS)

    Huang, Feng; Xu, Ju; Chen, Daqin; Wang, Yuansheng

    2012-10-01

    In this communication, a thermolysis route is developed to synthesize novel Cu1.94S-ZnS-Cu1.94S nanoheterostructures with interesting sandwich-like architectures, taking Cu1.94S nanoplates as precursors. Evidently, the trimeric nanostructure is formed by a three-stage process, which includes the Zn-oleate induced assembling of Cu1.94S nanoplate couples, the heteronucleation and growth of a ZnS layer between two Cu1.94S plates dominated by interfacial diffusion, and the catalyst assisted axial growth of ZnS nanorod following the solution-liquid-solid mechanism. With epitaxial growth of ZnS nanocrystal between two Cu1.94S nanoplates, the localized surface plasmon resonance frequency of Cu1.94S shifts from 1875 to 1323 nm, indicating that this new material is potentially applicable as a light absorbing agent in laser photothermal therapy. The reported growth mechanism may provide new strategies for designing and fabricating various technologically important polymeric nanoheterostructures.

  1. Resonance Trapping in Planetary Systems

    NASA Astrophysics Data System (ADS)

    Pour, Nader H.

    1998-09-01

    We study dynamics of a planetary system that consists of a star and two planets taking into account dynamical friction. Numerical integrations of a restricted planar circular three body model of this system indicate resonance capture. The main purpose of this paper is to present the results of an extensive numerical experiment performed on this model and also to present analytical arguments for the observed resonance trapping and its consequences. The equations of motion are written in terms of Delaunay variables and the recently developed method of partial averaging near resonance* is employed in order to account for the behavior of the system at resonance. * C.Chicone, B.Mashhoon and D.Retzloff, Ann.Inst.Henri Poincare, Vol.64, no 1, 1996, p.87-125.

  2. Functional Magnetic Resonance Imaging and Pediatric Anxiety

    ERIC Educational Resources Information Center

    Pine, Daniel S.; Guyer, Amanda E.; Leibenluft, Ellen; Peterson, Bradley S.; Gerber, Andrew

    2008-01-01

    The use of functional magnetic resonance imaging in investigating pediatric anxiety disorders is studied. Functional magnetic resonance imaging can be utilized in demonstrating parallels between the neural architecture of difference in anxiety of humans and the neural architecture of attention-orienting behavior in nonhuman primates or rodents.…

  3. Tunable Micro- and Nanomechanical Resonators

    PubMed Central

    Zhang, Wen-Ming; Hu, Kai-Ming; Peng, Zhi-Ke; Meng, Guang

    2015-01-01

    Advances in micro- and nanofabrication technologies have enabled the development of novel micro- and nanomechanical resonators which have attracted significant attention due to their fascinating physical properties and growing potential applications. In this review, we have presented a brief overview of the resonance behavior and frequency tuning principles by varying either the mass or the stiffness of resonators. The progress in micro- and nanomechanical resonators using the tuning electrode, tuning fork, and suspended channel structures and made of graphene have been reviewed. We have also highlighted some major influencing factors such as large-amplitude effect, surface effect and fluid effect on the performances of resonators. More specifically, we have addressed the effects of axial stress/strain, residual surface stress and adsorption-induced surface stress on the sensing and detection applications and discussed the current challenges. We have significantly focused on the active and passive frequency tuning methods and techniques for micro- and nanomechanical resonator applications. On one hand, we have comprehensively evaluated the advantages and disadvantages of each strategy, including active methods such as electrothermal, electrostatic, piezoelectrical, dielectric, magnetomotive, photothermal, mode-coupling as well as tension-based tuning mechanisms, and passive techniques such as post-fabrication and post-packaging tuning processes. On the other hand, the tuning capability and challenges to integrate reliable and customizable frequency tuning methods have been addressed. We have additionally concluded with a discussion of important future directions for further tunable micro- and nanomechanical resonators. PMID:26501294

  4. Tunable micro- and nanomechanical resonators.

    PubMed

    Zhang, Wen-Ming; Hu, Kai-Ming; Peng, Zhi-Ke; Meng, Guang

    2015-01-01

    Advances in micro- and nanofabrication technologies have enabled the development of novel micro- and nanomechanical resonators which have attracted significant attention due to their fascinating physical properties and growing potential applications. In this review, we have presented a brief overview of the resonance behavior and frequency tuning principles by varying either the mass or the stiffness of resonators. The progress in micro- and nanomechanical resonators using the tuning electrode, tuning fork, and suspended channel structures and made of graphene have been reviewed. We have also highlighted some major influencing factors such as large-amplitude effect, surface effect and fluid effect on the performances of resonators. More specifically, we have addressed the effects of axial stress/strain, residual surface stress and adsorption-induced surface stress on the sensing and detection applications and discussed the current challenges. We have significantly focused on the active and passive frequency tuning methods and techniques for micro- and nanomechanical resonator applications. On one hand, we have comprehensively evaluated the advantages and disadvantages of each strategy, including active methods such as electrothermal, electrostatic, piezoelectrical, dielectric, magnetomotive, photothermal, mode-coupling as well as tension-based tuning mechanisms, and passive techniques such as post-fabrication and post-packaging tuning processes. On the other hand, the tuning capability and challenges to integrate reliable and customizable frequency tuning methods have been addressed. We have additionally concluded with a discussion of important future directions for further tunable micro- and nanomechanical resonators.

  5. Magnetostriction and thermal expansion of the Kondo semiconductor Ce{sub 3}Bi{sub 4}Pt{sub 3}

    SciTech Connect

    Hundley, M.F.; Neumeier, J.J.; Thompson, J.D.; Lacerda, A.; Canfield, P.C.

    1995-05-01

    We report dilatometric thermal expansion ({alpha}) and magnetostriction ({lambda}) measurements on the Kondo semiconductor Ce{sub 3}Bi{sub 4}Pt{sub 3} and its non-magnetic analog La{sub 3}Bi{sub 4}Pt{sub 3} in fields to 100 kOe. The magnetic contribution to the thermal expansion of Ce{sub 3}Bi{sub 4}Pt{sub 3} displays a broad maximum centered at 50 K, close to the temperature where the 4f specific heat is a maximum. The linear magnetostriction is anomalously large in Ce{sub 3}Bi{sub 4}Pt{sub 3}, with values that are characteristic of mixed-valent compounds ({lambda}{sub {perpendicular}} = 3.26x10{sup {minus}5}, {lambda}{sub {parallel}} = -6.24x10{sup {minus}5} in 100 kOe at 4 K). The volume magnetostriction is positive and a factor of ten smaller than the linear coefficients ({lambda}{sub V} = 2.75x10{sup {minus}6} in 100 kOe at 4 K). The volume magnetostriction is temperature-dependent, and peaks at 50 K. The data are considered in terms of a Grueneisen analysis that links the temperature-dependent magnetic susceptibility, thermal expansion, magnetostriction, bulk modulus, and specific heat of Ce{sub 3}Bi{sub 4}Pt{sub 3} via temperature-dependent electronic and magnetic scaling parameters.

  6. Unusual Kondo-hole effect and crystal-field frustration in Nd-doped CeRhIn5

    NASA Astrophysics Data System (ADS)

    Rosa, P. F. S.; Oostra, A.; Thompson, J. D.; Pagliuso, P. G.; Fisk, Z.

    2016-07-01

    We investigate single crystals of Ce1 -xNdxRhIn5 by means of x-ray-diffraction, microprobe, magnetic susceptibility, heat capacity, and electrical resistivity measurements. Our data reveal that the antiferromagnetic transition of CeRhIn5, at TNCe=3.8 K, is linearly suppressed with xNd. We associate this effect with the presence of a "Kondo hole" created by Nd substitution. The extrapolation of TNCe to zero temperature, however, occurs at xc˜0.3 , which is below the two-dimensional percolation limit found in Ce1 -xLaxRhIn5 . This result strongly suggests the presence of a crystal-field induced magnetic frustration. Near xNd˜0.2 , the Ising antiferromagnetic order from Nd3 + ions is stabilized and TNNd increases up to 11 K in NdRhIn5. Our results shed light on the effects of magnetic doping in heavy-fermion antiferromagnets and stimulate the study of such systems under applied pressure.

  7. Three-dimensional bulk electronic structure of the Kondo lattice CeIn3 revealed by photoemission

    PubMed Central

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Liu, Qin; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Liu, Yu; Song, Haifeng; Zhang, Zhengjun; Lai, Xinchun

    2016-01-01

    We show the three-dimensional electronic structure of the Kondo lattice CeIn3 using soft x-ray angle resolved photoemission spectroscopy in the paramagnetic state. For the first time, we have directly observed the three-dimensional topology of the Fermi surface of CeIn3 by photoemission. The Fermi surface has a complicated hole pocket centred at the Γ-Z line and an elliptical electron pocket centred at the R point of the Brillouin zone. Polarization and photon-energy dependent photoemission results both indicate the nearly localized nature of the 4f electrons in CeIn3, consistent with the theoretical prediction by means of the combination of density functional theory and single-site dynamical mean-field theory. Those results illustrate that the f electrons of CeIn3, which is the parent material of CeMIn5 compounds, are closer to the localized description than the layered CeMIn5 compounds. PMID:27641364

  8. Insulator-to-metal transition in vanadium supersaturated silicon: variable-range hopping and Kondo effect signatures

    NASA Astrophysics Data System (ADS)

    García-Hemme, E.; Montero, D.; García-Hernansanz, R.; Olea, J.; Mártil, I.; González-Díaz, G.

    2016-07-01

    We report the observation of the insulator-to-metal transition in crystalline silicon samples supersaturated with vanadium. Ion implantation followed by pulsed laser melting and rapid resolidification produce high quality single-crystalline silicon samples with vanadium concentrations that exceed equilibrium values in more than 5 orders of magnitude. Temperature-dependent analysis of the conductivity and Hall mobility values for temperatures from 10 K to 300 K indicate that a transition from an insulating to a metallic phase is obtained at a vanadium concentration between 1.1  ×  1020 and 1.3  ×  1021 cm-3. Samples in the insulating phase present a variable-range hopping transport mechanism with a Coulomb gap at the Fermi energy level. Electron wavefunction localization length increases from 61 to 82 nm as the vanadium concentration increases in the films, supporting the theory of impurity band merging from delocalization of levels states. On the metallic phase, electronic transport present a dispersion mechanism related with the Kondo effect, suggesting the presence of local magnetic moments in the vanadium supersaturated silicon material.

  9. Interplay of atomic randomness and Kondo effect in disordered metallic conductor La2NiSi3.

    PubMed

    Gnida, Daniel; Szlawska, Maria; Swatek, Przemysław; Kaczorowski, Dariusz

    2016-11-01

    A polycrystalline sample of La2NiSi3 was investigated by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity and magnetoresistivity measurements. The compound was basically characterized as a Pauli paramagnet with metallic-like electrical conductivity, notably reduced in magnitude and weakly temperature dependent, as is usually observed for atomically disordered systems. Furthermore, the experimental data revealed the presence of a small amount of paramagnetic impurities. As a result, the low-temperature electrical resistivity in La2NiSi3 was found to be governed by both quantum corrections due to electron-electron interactions ([Formula: see text] contribution) and spin-flip Kondo scattering ([Formula: see text] contribution). The presence of paramagnetic impurities led to an increase in s-electron spin splitting due to the s-d interactions, manifested by a B (1/2) dependence of the magnetoresistivity, anomalously observed in the present study for thermal energy being larger than the Zeeman splitting energy [Formula: see text]. PMID:27603776

  10. Interplay of atomic randomness and Kondo effect in disordered metallic conductor La2NiSi3

    NASA Astrophysics Data System (ADS)

    Gnida, Daniel; Szlawska, Maria; Swatek, Przemysław; Kaczorowski, Dariusz

    2016-11-01

    A polycrystalline sample of La2NiSi3 was investigated by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity and magnetoresistivity measurements. The compound was basically characterized as a Pauli paramagnet with metallic-like electrical conductivity, notably reduced in magnitude and weakly temperature dependent, as is usually observed for atomically disordered systems. Furthermore, the experimental data revealed the presence of a small amount of paramagnetic impurities. As a result, the low-temperature electrical resistivity in La2NiSi3 was found to be governed by both quantum corrections due to electron-electron interactions (ρ ˜ {{T}1/2} contribution) and spin-flip Kondo scattering (ρ ˜ log T contribution). The presence of paramagnetic impurities led to an increase in s-electron spin splitting due to the s-d interactions, manifested by a B 1/2 dependence of the magnetoresistivity, anomalously observed in the present study for thermal energy being larger than the Zeeman splitting energy {{k}\\text{B}}T>g{μ\\text{B}}B .

  11. Three-dimensional bulk electronic structure of the Kondo lattice CeIn3 revealed by photoemission.

    PubMed

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Liu, Qin; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Liu, Yu; Song, Haifeng; Zhang, Zhengjun; Lai, Xinchun

    2016-01-01

    We show the three-dimensional electronic structure of the Kondo lattice CeIn3 using soft x-ray angle resolved photoemission spectroscopy in the paramagnetic state. For the first time, we have directly observed the three-dimensional topology of the Fermi surface of CeIn3 by photoemission. The Fermi surface has a complicated hole pocket centred at the Γ-Z line and an elliptical electron pocket centred at the R point of the Brillouin zone. Polarization and photon-energy dependent photoemission results both indicate the nearly localized nature of the 4f electrons in CeIn3, consistent with the theoretical prediction by means of the combination of density functional theory and single-site dynamical mean-field theory. Those results illustrate that the f electrons of CeIn3, which is the parent material of CeMIn5 compounds, are closer to the localized description than the layered CeMIn5 compounds. PMID:27641364

  12. Three-dimensional bulk electronic structure of the Kondo lattice CeIn3 revealed by photoemission

    NASA Astrophysics Data System (ADS)

    Zhang, Yun; Lu, Haiyan; Zhu, Xiegang; Tan, Shiyong; Liu, Qin; Chen, Qiuyun; Feng, Wei; Xie, Donghua; Luo, Lizhu; Liu, Yu; Song, Haifeng; Zhang, Zhengjun; Lai, Xinchun

    2016-09-01

    We show the three-dimensional electronic structure of the Kondo lattice CeIn3 using soft x-ray angle resolved photoemission spectroscopy in the paramagnetic state. For the first time, we have directly observed the three-dimensional topology of the Fermi surface of CeIn3 by photoemission. The Fermi surface has a complicated hole pocket centred at the Γ-Z line and an elliptical electron pocket centred at the R point of the Brillouin zone. Polarization and photon-energy dependent photoemission results both indicate the nearly localized nature of the 4f electrons in CeIn3, consistent with the theoretical prediction by means of the combination of density functional theory and single-site dynamical mean-field theory. Those results illustrate that the f electrons of CeIn3, which is the parent material of CeMIn5 compounds, are closer to the localized description than the layered CeMIn5 compounds.

  13. Space charge effects: tune shifts and resonances

    SciTech Connect

    Weng, W.T.

    1986-08-01

    The effects of space charge and beam-beam interactions on single particle motion in the transverse degree of freedom are considered. The space charge force and the resulting incoherent tune shift are described, and examples are given from the AGS and CERN's PSB. Equations of motion are given for resonances in the presence of the space charge force, and particle behavior is examined under resonance and space charge conditions. Resonance phase space structure is described with and without space charge. Uniform and bunched beams are compared. Beam-beam forces and resonances and beam-beam detuning are described. 18 refs., 15 figs. (LEW)

  14. Universal transport signatures in two-electron molecular quantum dots: gate-tunable Hund's rule, underscreened Kondo effect and quantum phase transitions

    NASA Astrophysics Data System (ADS)

    Florens, Serge; Freyn, Axel; Roch, Nicolas; Wernsdorfer, Wolfgang; Balestro, Franck; Roura-Bas, Pablo; Aligia, A. A.

    2011-06-01

    We review here some universal aspects of the physics of two-electron molecular transistors in the absence of strong spin-orbit effects. Several recent quantum dot experiments have shown that an electrostatic backgate could be used to control the energy dispersion of magnetic levels. We discuss how the generally asymmetric coupling of the metallic contacts to two different molecular orbitals can indeed lead to a gate-tunable Hund's rule in the presence of singlet and triplet states in the quantum dot. For gate voltages such that the singlet constitutes the (non-magnetic) ground state, one generally observes a suppression of low voltage transport, which can yet be restored in the form of enhanced cotunneling features at finite bias. More interestingly, when the gate voltage is controlled to obtain the triplet configuration, spin S = 1 Kondo anomalies appear at zero bias, with non-Fermi liquid features related to the underscreening of a spin larger than 1/2. Finally, the small bare singlet-triplet splitting in our device allows fine-tuning with the gate between these two magnetic configurations, leading to an unscreening quantum phase transition. This transition occurs between the non-magnetic singlet phase, where a two-stage Kondo effect occurs, and the triplet phase, where the partially compensated (underscreened) moment is akin to a magnetically 'ordered' state. These observations are put theoretically into a consistent global picture by using new numerical renormalization group simulations, tailored to capture sharp finite-voltage cotunneling features within the Coulomb diamonds, together with complementary out-of-equilibrium diagrammatic calculations on the two-orbital Anderson model. This work should shed further light on the complicated puzzle still raised by multi-orbital extensions of the classic Kondo problem.

  15. A Comparison of Magnetic Resonance Imaging and Neuropsychological Examination in the Diagnostic Distinction of Alzheimer's Disease and Behavioral Variant Frontotemporal Dementia.

    PubMed

    Wang, Jingjing; Redmond, Stephen J; Bertoux, Maxime; Hodges, John R; Hornberger, Michael

    2016-01-01

    The clinical distinction between Alzheimer's disease (AD) and behavioral variant frontotemporal dementia (bvFTD) remains challenging and largely dependent on the experience of the clinician. This study investigates whether objective machine learning algorithms using supportive neuroimaging and neuropsychological clinical features can aid the distinction between both diseases. Retrospective neuroimaging and neuropsychological data of 166 participants (54 AD; 55 bvFTD; 57 healthy controls) was analyzed via a Naïve Bayes classification model. A subgroup of patients (n = 22) had pathologically-confirmed diagnoses. Results show that a combination of gray matter atrophy and neuropsychological features allowed a correct classification of 61.47% of cases at clinical presentation. More importantly, there was a clear dissociation between imaging and neuropsychological features, with the latter having the greater diagnostic accuracy (respectively 51.38 vs. 62.39%). These findings indicate that, at presentation, machine learning classification of bvFTD and AD is mostly based on cognitive and not imaging features. This clearly highlights the urgent need to develop better biomarkers for both diseases, but also emphasizes the value of machine learning in determining the predictive diagnostic features in neurodegeneration. PMID:27378905

  16. Behavior of cholesterol and spin-labeled cholestane in model bile systems studied by electron spin resonance and synchrotron x-ray.

    PubMed Central

    Sömjen, G. J.; Lipka, G.; Schulthess, G.; Koch, M. H.; Wachtel, E.; Gilat, T.; Hauser, H.

    1995-01-01

    The behavior of mixed bile salt micelles consisting of sodium taurocholate, egg phosphatidylcholine, and cholesterol has been studied by ESR spin labeling and synchrotron x-ray scattering. Consistent with published phase diagrams, pure and mixed bile salt micelles have a limited capacity to incorporate and, hence, solubilize cholesterol. Excess cholesterol crystallizes out, a process that is readily detected both by ESR spin labeling using 3-doxyl-5 alpha-cholestane as a probe for cholesterol and synchrotron x-ray scattering. Both methods yield entirely consistent results. The crystallization of cholesterol from mixed bile salt micelles is indicated by the appearance of a magnetically dilute powder spectrum that is readily detected by visual inspection of the ESR spectra. Both the absence of Heissenberg spin exchange and the observation of a magnetically dilute powder spectrum provide evidence for the spin label co-crystallizing with cholesterol. In mixed bile salt micelles containing egg phosphatidylcholine, the solubility of cholesterol is increased as detected by both methods. With increasing content of phosphatidylcholine and increasing mole ratio cholesterol/phosphatidylcholine, the anisotropy of motion of the spin probe increases. The spin label 3-doxyl-5 alpha-cholestane is a useful substitute for cholesterol provided that it is used in dilute mixtures with excess cholesterol: the cholesterol/spin label mole ratio in these mixtures should be greater than 100. Despite the structural similarity between the two compounds, there are still significant differences in their physico-chemical properties. These differences come to the fore when cholesterol is totally replaced by the spin-label: 3-doxyl-5a-cholestane is significantly less soluble in bile salt and mixed bile salt micelles than cholesterol and, in contrast with cholesterol, it interacts only very weakly, if at all,with phosphatidylcholine. The potential of the ESR method for detecting cholesterol crystal

  17. Neutron diffraction study of magnetic field induced behavior in the heavy Fermion Ce3Co4Sn13

    SciTech Connect

    Christianson, Andrew D; Goremychkin, E. A.; Gardner, J. S.; Kang, H. J.; Chung, J.-H.; Manuel, P.; Thompson, J. D.; Sarrao, J. L.; Lawrence, J. M.

    2008-01-01

    The specific heat of Ce3Co4Sn13 exhibits a crossover from heavy Fermion behavior with antiferromagnetic correlations at low field to single impurity Kondo behavior above 2 T. We have performed neutron diffraction measurements in magnetic fields up to 6 Tesla on single crystal samples. The (001) position shows a dramatic increase in intensity in field which appears to arise from static polarization of the 4f level and which at 0.14 K also exhibits an anomaly near 2T reflecting the crossover to single impurity behavior.

  18. Hall effect anomaly and low-temperature metamagnetism in the Kondo compound CeAgBi2

    NASA Astrophysics Data System (ADS)

    Thomas, S. M.; Rosa, P. F. S.; Lee, S. B.; Parameswaran, S. A.; Fisk, Z.; Xia, J.

    2016-02-01

    Heavy fermion (HF) materials exhibit a rich array of phenomena due to the strong Kondo coupling between their localized moments and itinerant electrons. A central question in their study is to understand the interplay between magnetic order and charge transport, and its role in stabilizing new quantum phases of matter. Particularly promising in this regard is a family of tetragonal intermetallic compounds Ce T X2 (where T denotes transition metal and X denotes pnictogen), which includes a variety of HF compounds showing T -linear electronic specific heat Ce˜γ T , with γ ˜20 -500 mJ mol-1K-2 , reflecting an effective-mass enhancement ranging from small to modest. Here, we study the low-temperature field-tuned phase diagram of high-quality CeAgBi2 using magnetometry and transport measurements. We find an antiferromagnetic transition at TN=6.4 K with weak magnetic anisotropy and the easy axis along the c axis, similar to previous reports (TN=6.1 K ). This scenario, along with the presence of two anisotropic Ruderman-Kittel-Kasuya-Yosida interactions, leads to a rich field-tuned magnetic phase diagram, consisting of five metamagnetic transitions of both first and second order. In addition, we unveil an anomalous Hall contribution for fields H <54 kOe , which is drastically altered when H is tuned through a trio of transitions at 57, 78, and 84 kOe, suggesting that the Fermi surface is reconstructed in a subset of the metamagnetic transitions.

  19. Design and characterization of a windowless resonant photoacoustic chamber equipped with resonance locking circuitry

    NASA Astrophysics Data System (ADS)

    Angeli, György Z.; Bozóki, Zoltán; Miklós, András; Lörincz, András; Thöny, Andreas; Sigrist, Markus W.

    1991-03-01

    A novel design of a windowless resonant photoacoustic chamber with open acoustic filters and an electronic resonance locking circuitry is presented. The acoustic behavior of the cell and preliminary measurements on a certified gas mixture with a CO2 laser demonstrate the feasibility for trace gas monitoring.

  20. Spin fluctuations and hidden-order phases in Ce-based Kondo systems

    NASA Astrophysics Data System (ADS)

    Inosov, D. S.; Portnichenko, P. Y.; Cameron, A. S.; Paschen, S.; Prokofiev, A.; Friemel, G.; Jang, H.; Keimer, B.; Filipov, V. B.; Shitsevalova, N. Y.; Schneidewind, A.; Ivanov, A.; Ollivier, J.; Deen, P. P.; Strydom, A. M.

    Among heavy-fermion metals, both CeB6 and Ce3Pd20Si6 compounds exhibit a magnetically hidden ordered phase in their low-temperature phase diagram, which is attributed to the ordering of magnetic quadrupolar moments, known as the antiferroquadrupolar (AFQ) ordering. Using inelastic neutron scattering, we have investigated the spectrum of spin excitations in both systems. In the structurally simplest CeB6, it consists of several contributions including conventional spin waves that coexist with both ferro- and antiferromagnetic excitonic resonance-like modes. However, the structurally more complex Ce3Pd20Si6 possesses a much simpler magnetic excitation spectrum with only a single contribution peaked around the AFQ wave vector. It remains quasielastic in the absence of an external magnetic field, but then develops into dispersive magnon modes whose band width scales linearly with the applied field. Furthermore, neutron diffraction measurements on the same sample at sub-Kelvin temperatures revealed diffuse magnetic scattering that can be associated with the hidden order parameter. Supported by DFG Grant No. IN 209/3-1.

  1. Experiments with Helmholtz Resonators.

    ERIC Educational Resources Information Center

    Greenslade, Thomas B., Jr.

    1996-01-01

    Presents experiments that use Helmholtz resonators and have been designed for a sophomore-level course in oscillations and waves. Discusses the theory of the Helmholtz resonator and resonance curves. (JRH)

  2. The genetic diversity,relationships,and potential for biological control of the lobate lac scale,Paratachardina pseudolobata Kondo&Gullan(Hemiptera:Coccoidea:Kerriidae),a pest in Florida,the Bahamas,Cuba and Christmas Island

    Technology Transfer Automated Retrieval System (TEKTRAN)

    The lobate lac scale Paratachardina pseudolobata Kondo & Gullan (Kerriidae) is a polyphagous pest of woody plants in Florida (U.S.A), the Bahamas, Cuba, and Christmas Island (Australia). Its recent appearance as a pest in these places indicates that this scale is introduced; however, its native rang...

  3. Regenerative feedback resonant circuit

    DOEpatents

    Jones, A. Mark; Kelly, James F.; McCloy, John S.; McMakin, Douglas L.

    2014-09-02

    A regenerative feedback resonant circuit for measuring a transient response in a loop is disclosed. The circuit includes an amplifier for generating a signal in the loop. The circuit further includes a resonator having a resonant cavity and a material located within the cavity. The signal sent into the resonator produces a resonant frequency. A variation of the resonant frequency due to perturbations in electromagnetic properties of the material is measured.

  4. Study of the magnetic properties of the Cex La1-x Pt alloy system: Which interaction establishes ferromagnetism in Kondo systems?

    NASA Astrophysics Data System (ADS)

    Očko, M.; Zadro, K.; Drobac, Đ.; Aviani, I.; Salamon, K.; Mixson, D.; Bauer, E. D.; Sarrao, J. L.

    2016-11-01

    In order to study Kondo ferromagnetism, particularly of the CePt compound, we investigate the magnetic properties of the CexLa1-xPt alloy system in the temperature range from 1.8 K to 320 K. The results of these investigations can be summarized as follows: dc-susceptibility can be described by the Curie-Weiss law at higher temperatures down to about 100 K, but also at the low temperatures above the phase transition. At higher temperatures, the extracted Curie-Weiss constant, θp, is negative in contrast to the low temperatures, where θC is positive. The extracted effective magnetic moment from the higher temperatures is the same for all the alloys and is close to the theoretical value of the isolated Ce3+ ion, μ=2.54 μB, indicating the hybridization is weak and, and consequently, Kondo interaction is weak. These observations confirm the main important conclusions inferred from an earlier transport properties investigation of this alloy system. The Curie temperature extracted by various approaches was compared to the extraction from the ac-susceptibility measurements. We show that its concentration dependence is not consistent with Doniach's diagram. Hence, RKKY interaction is not responsible for the ferromagnetism in this alloy system.

  5. Triad mode resonant interactions in suspended cables

    NASA Astrophysics Data System (ADS)

    Guo, TieDing; Kang, HouJun; Wang, LianHua; Zhao, YueYu

    2016-03-01

    A triad mode resonance, or three-wave resonance, is typical of dynamical systems with quadratic nonlinearities. Suspended cables are found to be rich in triad mode resonant dynamics. In this paper, modulation equations for cable's triad resonance are formulated by the multiple scale method. Dynamic conservative quantities, i.e., mode energy and Manley-Rowe relations, are then constructed. Equilibrium/dynamic solutions of the modulation equations are obtained, and full investigations into their stability and bifurcation characteristics are presented. Various bifurcation behaviors are detected in cable's triad resonant responses, such as saddle-node, Hopf, pitchfork and period-doubling bifurcations. Nonlinear behaviors, like jump and saturation phenomena, are also found in cable's responses. Based upon the bifurcation analysis, two interesting properties associated with activation of cable's triad resonance are also proposed, i.e., energy barrier and directional dependence. The first gives the critical amplitude of high-frequency mode to activate cable's triad resonance, and the second characterizes the degree of difficulty for activating cable's triad resonance in two opposite directions, i.e., with positive or negative internal detuning parameter.

  6. Electroexcitation of nucleon resonances

    SciTech Connect

    Inna Aznauryan, Volker D. Burkert

    2012-01-01

    We review recent progress in the investigation of the electroexcitation of nucleon resonances, both in experiment and in theory. The most accurate results have been obtained for the electroexcitation amplitudes of the four lowest excited states, which have been measured in a range of Q2 up to 8 and 4.5 GeV2 for the Delta(1232)P33, N(1535)S11 and N(1440)P11, N(1520)D13, respectively. These results have been confronted with calculations based on lattice QCD, large-Nc relations, perturbative QCD (pQCD), and QCD-inspired models. The amplitudes for the Delta(1232) indicate large pion-cloud contributions at low Q2 and don't show any sign of approaching the pQCD regime for Q2<7 GeV2. Measured for the first time, the electroexcitation amplitudes of the Roper resonance, N(1440)P11, provide strong evidence for this state as a predominantly radial excitation of a three-quark (3q) ground state, with additional non-3-quark contributions needed to describe the low Q2 behavior of the amplitudes. The longitudinal transition amplitude for the N(1535)S11 was determined and has become a challenge for quark models. Explanations may require large meson-cloud contributions or alternative representations of this state. The N(1520)D13 clearly shows the rapid changeover from helicity-3/2 dominance at the real photon point to helicity-1/2 dominance at Q2 > 0.5 GeV2, confirming a long-standing prediction of the constituent quark model. The interpretation of the moments of resonance transition form factors in terms of transition transverse charge distributions in infinite momentum frame is presented.

  7. Basics of magnetic resonance imaging

    SciTech Connect

    Oldendorf, W.; Oldendorf, W. Jr.

    1988-01-01

    Beginning with the behavior of a compass needle in a magnetic field, this text uses analogies from everyday experience to explain the phenomenon of nuclear magnetic resonance and how it is used for imaging. Using a minimum of scientific abbreviations and symbols, the basics of tissue visualization and characterization are presented. A description of the various types of magnets and scanners is followed by the practical advantages and limitations of MRI relative to x-ray CT scanning.

  8. Distributed Hybridization Model for Quantum Critical Behavior in Magnetic Quasicrystals

    NASA Astrophysics Data System (ADS)

    Otsuki, Junya; Kusunose, Hiroaki

    2016-07-01

    A quantum critical behavior of the magnetic susceptibility was observed in a quasicrystal containing ytterbium. At the same time, a mixed-valence feature of Yb ions was reported, which appears to be incompatible with the magnetic instability. We derive the magnetic susceptibility by expressing the quasiperiodicity as the distributed hybridization strength between Yb 4f and conduction electrons. Assuming a wide distribution of the hybridization strength, the most f electrons behave as renormalized paramagnetic states in the Kondo or mixed-valence regime, but a small number of f moments remain unscreened. As a result, the bulk magnetic susceptibility exhibits a nontrivial power-law-like behavior, while the average f-electron occupation is that of mixed-valence systems. This model thus resolves two contradictory properties of Yb quasicrystals.

  9. A preclinical murine model for the early detection of radiation-induced brain injury using magnetic resonance imaging and behavioral tests for learning and memory: with applications for the evaluation of possible stem cell imaging agents and therapies.

    PubMed

    Ngen, Ethel J; Wang, Lee; Gandhi, Nishant; Kato, Yoshinori; Armour, Michael; Zhu, Wenlian; Wong, John; Gabrielson, Kathleen L; Artemov, Dmitri

    2016-06-01

    Stem cell therapies are being developed for radiotherapy-induced brain injuries (RIBI). Magnetic resonance imaging (MRI) offers advantages for imaging transplanted stem cells. However, most MRI cell-tracking techniques employ superparamagnetic iron oxide particles (SPIOs), which are difficult to distinguish from hemorrhage. In current preclinical RIBI models, hemorrhage occurs concurrently with other injury markers. This makes the evaluation of the recruitment of transplanted SPIO-labeled stem cells to injury sites difficult. Here, we developed a RIBI model, with early injury markers reflective of hippocampal dysfunction, which can be detected noninvasively with MRI and behavioral tests. Lesions were generated by sub-hemispheric irradiation of mouse hippocampi with single X-ray beams of 80 Gy. Lesion formation was monitored with anatomical and contrast-enhanced MRI and changes in memory and learning were assessed with fear-conditioning tests. Early injury markers were detected 2 weeks after irradiation. These included an increase in the permeability of the blood-brain barrier, demonstrated by a 92 ± 20 % contrast enhancement of the irradiated versus the non-irradiated brain hemispheres, within 15 min of the administration of an MRI contrast agent. A change in short-term memory was also detected, as demonstrated by a 40.88 ± 5.03 % decrease in the freezing time measured during the short-term memory context test at this time point, compared to that before irradiation. SPIO-labeled stem cells transplanted contralateral to the lesion migrated toward the lesion at this time point. No hemorrhage was detected up to 10 weeks after irradiation. This model can be used to evaluate SPIO-based stem cell-tracking agents, short-term. PMID:27021492

  10. Cavity- and waveguide-resonators in electron paramagnetic resonance, nuclear magnetic resonance, and magnetic resonance imaging.

    PubMed

    Webb, Andrew

    2014-11-01

    Cavity resonators are widely used in electron paramagnetic resonance, very high field magnetic resonance microimaging and also in high field human imaging. The basic principles and designs of different forms of cavity resonators including rectangular, cylindrical, re-entrant, cavity magnetrons, toroidal cavities and dielectric resonators are reviewed. Applications in EPR and MRI are summarized, and finally the topic of traveling wave MRI using the magnet bore as a waveguide is discussed.

  11. Implementation and characterization of meta-resonator antennas

    NASA Astrophysics Data System (ADS)

    Kim, In Kwang; Varadan, Vasundara V.

    2015-04-01

    Metamaterials are artificially engineered microstructures that have strong resonance behavior although their electrical size is very small. Meta-resonator (metamaterial resonator) antennas use the resonance of the metamaterials to reduce the size of radiators and design multiband antennas. A split-ring resonator (SRR) is a well-studied metamaterial structure which obtains negative permittivity and/or permeability in a narrow frequency region. In this paper, metamaterial structures and meta-resonator antennas are designed and simulated using a full wave simulator. 2D metaresonator antennas are fabricated by photolithography and 3D meta-resonator antennas are fabricated by LTCC (Low- Temperature Co-fired Ceramic) technique. A free space measurement system is used to characterize metamaterial samples. Several 2D/3D meta-resonator antennas with SRRs are described.

  12. Resonant Anderson localization in segmented wires.

    PubMed

    Estarellas, Cristian; Serra, Llorenç

    2016-03-01

    We discuss a model of random segmented wire, with linear segments of two-dimensional wires joined by circular bends. The joining vertices act as scatterers on the propagating electron waves. The model leads to resonant Anderson localization when all segments are of similar length. The resonant behavior is present with one and also with several propagating modes. The probability distributions evolve from diffusive to localized regimes when increasing the number of segments in a similar way for long and short localization lengths. As a function of the energy, a finite segmented wire typically evolves from localized to diffusive to ballistic behavior in each conductance plateau.

  13. Magnetic structure of the antiferromagnetic Kondo lattice compounds CeRhAl4Si2 and CeIrAl4Si2

    DOE PAGES

    Ghimire, N. J.; Calder, S.; Janoschek, M.; Bauer, E. D.

    2015-06-01

    In this article, we have investigated the magnetic ground state of the antiferromagnetic Kondo-lattice compounds CeMAl4Si2(M = Rh, Ir) using neutron powder diffraction. Although both of these compounds show two magnetic transitions TN1 and TN2 in the bulk properties measurements, evidence for magnetic long-range order was only found below the lower transition TN2. Analysis of the diffraction profiles reveals a commensurate antiferromagnetic structure with a propagation vector k = (0, 0, 1/2). The magnetic moment in the ordered state of CeRhAl4Si2 and CeIrAl4Si2 were determined to be 1.14(2) and 1.41(3) μB/Ce, respectively, and are parallel to the crystallographic c-axis inmore » agreement with magnetic susceptibility measurements.« less

  14. Kondo Lattice Effects of YbAl3 Suggested by Temperature Dependence of High-Accuracy High-Energy Photoelectron Spectroscopy

    NASA Astrophysics Data System (ADS)

    Suga, Shigemasa; Sekiyama, Akira; Imada, Shin; Shigemoto, Akihiko; Yamasaki, Atsushi; Tsunekawa, Masanori; Dallera, Claudia; Braicovich, Lucio; Lee, Tien-Lin; Sakai, Osamu; Ebihara, Takao; Ōnuki, Yoshichika

    2005-11-01

    By use of high-resolution soft X-rays, intrinsic temperature dependences of bulk Yb 4f photoelectron spectra were obtained for fractured surfaces of high-purity YbAl3 single crystals. The spectra of not only bulk 4f13 but also 4f12 final states are analyzed by noncrossing approximation (NCA) calculation for the f14, f13, and f12 initial states based on the single impurity Anderson model (SIAM). In order to consistently interpret the temperature dependences of both 4f13 and 4f12 final states, however, it is found that a constant set of parameters of the hybridization strength Δ, bare 4f energy \\varepsilonf and electron correlation energy Uff is insufficient. The limitation of SIAM is confirmed for YbAl3 and the importance of the Kondo lattice effects is suggested.

  15. Integral resonator gyroscope

    NASA Technical Reports Server (NTRS)

    Shcheglov, Kirill V. (Inventor); Challoner, A. Dorian (Inventor); Hayworth, Ken J. (Inventor); Wiberg, Dean V. (Inventor); Yee, Karl Y. (Inventor)

    2008-01-01

    The present invention discloses an inertial sensor having an integral resonator. A typical sensor comprises a planar mechanical resonator for sensing motion of the inertial sensor and a case for housing the resonator. The resonator and a wall of the case are defined through an etching process. A typical method of producing the resonator includes etching a baseplate, bonding a wafer to the etched baseplate, through etching the wafer to form a planar mechanical resonator and the wall of the case and bonding an end cap wafer to the wall to complete the case.

  16. Does Long-Term High Fat Diet Always Lead to Smaller Hippocampi Volumes, Metabolite Concentrations, and Worse Learning and Memory? A Magnetic Resonance and Behavioral Study in Wistar Rats

    PubMed Central

    Setkowicz, Zuzanna; Gaździńska, Agata; Osoba, Joanna J.; Karwowska, Karolina; Majka, Piotr; Orzeł, Jarosław; Kossowski, Bartosz; Bogorodzki, Piotr; Janeczko, Krzysztof; Wyleżoł, Mariusz; Gazdzinski, Stefan P.

    2015-01-01

    Background Obesity is a worldwide epidemic with more than 600 million affected individuals. Human studies have demonstrated some alterations in brains of otherwise healthy obese individuals and elevated risk of neurodegenerative disease of old age; these studies have also pointed to slightly diminished memory and executive functions among healthy obese individuals. Similar findings were obtained in animal models of obesity induced by high fat diet. On the other hand, low carbohydrate high fat diets are currently promoted for losing weight (e.g., Atkin’s style diets). However, the long-term effects of such diets are not known. Additionally, high fat diets leading to (mild) ketonemia were shown to improve brain function in elderly humans and in some animal models. Aim To evaluate the hypothesis that long-term use of a high fat diet was associated with decreases in spatial memory, smaller hippocampi and hippocampi metabolite concentrations in Wistar rats. Methods Twenty five male Wistar rats were put on high fat diet (HFD; 60% calories from fat, 30% from carbohydrates) on their 55th day of life, while 25 control male rats (CONs) remained on chow. Adequate levels of essential nutrients were provided. Both groups underwent memory tests in 8-arm radial maze at 3rd, 6th, 9th, and 12th month. 1H magnetic resonance spectroscopy was employed to measure concentrations of tNAA (marker of neuronal integrity) at one month and one year, whereas MRI was used to evaluate hippocampal volumes. Results Obese rats (OBRs) consumed similar amount of calories as CONs, but less proteins. However, their protein intake was within recommended amounts. Throughout the experiment OBRs had statistically higher concentrations of blood ketone bodies than CONs, but still within normal values. At post-mortem assessment, OBRs had 38% larger fat deposits than CONs (p<0.05), as evaluated by volume of epididymis fat, an acknowledged marker of fat deposits in rats. Contrary to our expectations, OBRs had

  17. Neutron resonance averaging

    SciTech Connect

    Chrien, R.E.

    1986-10-01

    The principles of resonance averaging as applied to neutron capture reactions are described. Several illustrations of resonance averaging to problems of nuclear structure and the distribution of radiative strength in nuclei are provided. 30 refs., 12 figs.

  18. Nanomechanical resonance detector

    DOEpatents

    Grossman, Jeffrey C; Zettl, Alexander K

    2013-10-29

    An embodiment of a nanomechanical frequency detector includes a support structure and a plurality of elongated nanostructures coupled to the support structure. Each of the elongated nanostructures has a particular resonant frequency. The plurality of elongated nanostructures has a range of resonant frequencies. An embodiment of a method of identifying an object includes introducing the object to the nanomechanical resonance detector. A resonant response by at least one of the elongated nanostructures of the nanomechanical resonance detector indicates a vibrational mode of the object. An embodiment of a method of identifying a molecular species of the present invention includes introducing the molecular species to the nanomechanical resonance detector. A resonant response by at least one of the elongated nanostructures of the nanomechanical resonance detector indicates a vibrational mode of the molecular species.

  19. Lattice Induced Resonances in One Dimensional Bosonic Systems

    NASA Astrophysics Data System (ADS)

    von Stecher, Javier; Gurarie, Victor; Radzihovsky, Leo; Rey, Ana Maria

    2011-05-01

    Feshbach resonances and optical lattices offer a unique opportunity for achieving new ways to control and explore novel many-body phenomena in strongly correlated atomic systems. To deal with such complex systems a natural prerequisite is a full understanding of the underlying two-body physics. Here, we investigate the lattice induced resonances produced when dimers formed with atoms in excited bands become resonant with the atoms in the lowest band. We first obtain accurate two-body solutions and demonstrate that the resonant effects depend strongly on the parity properties of the dimer. Then, we develop a novel two-channel effective lattice Hamiltonian with a parity dependent atom-dimer coupling that provides a starting point to analyze the many-body behavior of the resonant lattice system. We conclude that the lattice induced resonances significantly affect the behavior of the atoms in the lowest band and can be used to tune lattice systems to novel many-body regimes.

  20. Vibrational resonance in Duffing systems with fractional-order damping.

    PubMed

    Yang, J H; Zhu, H

    2012-03-01

    The phenomenon of vibrational resonance (VR) is investigated in over- and under-damped Duffing systems with fractional-order damping. It is found that the factional-order damping can induce change in the number of the steady stable states and then lead to single- or double-resonance behavior. Compared with vibrational resonance in the ordinary systems, the following new results are found in the fractional-order systems. (1) In the overdamped system with double-well potential and ordinary damping, there is only one kind of single-resonance, whereas there are double-resonance and two kinds of single-resonance for the case of fractional-order damping. The necessary condition for these new resonance behaviors is the value of the fractional-order satisfies α > 1. (2) In the overdamped system with single-well potential and ordinary damping, there is no resonance, whereas there is a single-resonance for the case of fractional-order damping. The necessary condition for the new result is α > 1. (3) In the underdamped system with double-well potential and ordinary damping, there are double-resonance and one kind of single-resonance, whereas there are double-resonance and two kinds of single-resonance for the case of fractional-order damping. The necessary condition for the new single-resonance is α < 1. (4) In the underdamped system with single-well potential, there is at most a single-resonance existing for both the cases of ordinary and fractional-order damping. In the underdamped systems, varying the value of the fractional-order is equivalent to change the damping parameter for some cases. PMID:22462988

  1. An Inexpensive Resonance Demonstration

    ERIC Educational Resources Information Center

    Dukes, Phillip

    2005-01-01

    The phenomenon of resonance is applicable to almost every branch of physics. Without resonance, there wouldn't be televisions or stereos, or even swings on the playground. However, resonance also has undesirable side effects such as irritating noises in the car and the catastrophic events such as helicopters flying apart. In this article, the…

  2. Fano resonance and the hidden order in URu2 Si 2 probed by quasiparticle scattering spectroscopy*

    NASA Astrophysics Data System (ADS)

    Park, W. K.; Greene, L. H.; Bauer, E. D.; Tobash, P. H.; Ronning, F.; Lu, X.; Sarrao, J. L.; Thompson, J. D.

    2011-03-01

    The nature of the hidden order transition occurring at 17.5 K in URu 2 Si 2 remains puzzling despite intensive investigations over the past two and half decades. Recent experimental and theoretical developments render it a timely subject to probe the hidden order state using quasiparticle tunneling and scattering techniques. We report on the Fano resonance in pure and Rh-doped URu 2 Si 2 single crystals using point-contact spectroscopy. The conductance spectra reproducibly reveal asymmetric double peak structures slightly off-centered around zero bias with the two peaks merging well above the hidden order transition temperature. An analysis using the Fano resonance model in a Kondo lattice [1] shows that the conductance peaks arise from the hybridization gap opening. Our estimated gap size agrees well with those reported from other measurements. We will present experimental results over a wide parameter space including temperature and doping dependences and discuss their underlying physics. M. Maltseva, M. Dzero, and P. Coleman, Phys. Rev. Lett. 103, 206402 (2009). * The work at UIUC is supported by the U.S. DOE under Award Nos. DE-FG02-07ER46453 and DE-AC02-98CH10886, and the work at LANL is carried out under the auspices of the U.S. DOE, Office of Science.

  3. Ovenized microelectromechanical system (MEMS) resonator

    SciTech Connect

    Olsson, Roy H; Wojciechowski, Kenneth; Kim, Bongsang

    2014-03-11

    An ovenized micro-electro-mechanical system (MEMS) resonator including: a substantially thermally isolated mechanical resonator cavity; a mechanical oscillator coupled to the mechanical resonator cavity; and a heating element formed on the mechanical resonator cavity.

  4. Visuomotor resonance in autism spectrum disorders.

    PubMed

    Becchio, Cristina; Castiello, Umberto

    2012-01-01

    When we observe the actions performed by others, our motor system "resonates" along with that of the observed agent. Is a similar visuomotor resonant response observed in autism spectrum disorders (ASD)? Studies investigating action observation in ASD have yielded inconsistent findings. In this perspective article we examine behavioral and neuroscientific evidence in favor of visuomotor resonance in ASD, and consider the possible role of action-perception coupling in social cognition. We distinguish between different aspects of visuomotor resonance and conclude that while some aspects may be preserved in ASD, abnormalities exist in the way individuals with ASD convert visual information from observed actions into a program for motor execution. Such abnormalities, we surmise, may contribute to but also depend on the difficulties that individuals with ASD encounter during social interaction.

  5. Subwavelength resonant nanostructured films for sensing

    SciTech Connect

    Alvine, Kyle J.; Bernacki, Bruce E.; Suter, Jonathan D.; Bennett, Wendy D.; Edwards, Daniel L.; Mendoza, Albert

    2013-05-29

    We present a novel subwavelength nanostructure architecture that may be utilized for optical standoff sensing applications. The subwavelength structures are fabricated via a combination of nanoimprint lithography and metal sputtering to create metallic nanostructured films encased within a transparent media. The structures are based on the open ring resonator (ORR) architecture and have their analog in resonant LC circuits, which display a resonance frequency that is inversely proportional to the square root of the product of the inductance and capacitance. Therefore, any perturbation of the nanostructured films due to chemical or environmental effects can alter the inductive or capacitive behavior of the subwavelength features, which can shift the resonant frequency and provide an indication of the external stimulus. This shift in resonance can be interrogated remotely either actively using either laser illumination or passively using hyperspectral or multispectral sensing. These structures may be designed to be either anisotropic or isotropic, which can also provide polarization-sensitive interrogation. Due to the nanometer-scale of the structures, they can be tailored to be optically responsive in the visible or near infrared spectrum with a highly reflective resonant peak that is dependent solely on structural dimensions and material characteristics. We present experimental measurements of the optical response of these structures as a function of wavelength, polarization, and incident angle demonstrating the resonant effect in the near infrared region. Numerical modeling data showing the effect of different fabrication parameters such as structure parameters are also discussed.

  6. Resonant discharge simulations with asymmetric electrodes

    SciTech Connect

    Smith, H.B.; Bowers, K.J.; Birdsall, C.K.

    1999-07-01

    Bounded plasmas exhibit two basic natural resonances--the plasma frequency and the series resonance frequency. The latter is associated with the edge of the plasma, and involves density perturbations in the sheath; it is also the cut-off frequency for waves propagating along the wall. Series resonant discharges have been previously simulated in planar 1d3v (one spatial dimension, 3 velocity dimensions) models. Results from these simulations are found to compare well with experimental measurements. In this paper the authors will look at 1d3v simulations of series resonant discharges between concentric cylinders and concentric spheres, also 1d3v. First, the natural series resonant frequency is determined by simulating an undriven plasma between short-circuited electrodes, looking for the resonance in the current; this frequency will be checked with simple circuit modeling. Second, they driven the same model near this resonance, in order to obtain a self-sustained discharge. They will report in detail on the differences between the driven symmetric and asymmetric discharges with respect to start-up, lock-on and steady state behavior, as well as on scaling laws.

  7. Quantum processes in resonators with moving walls

    NASA Technical Reports Server (NTRS)

    Klimov, A. B.; Dodonov, V. V.

    1993-01-01

    The behavior of an electromagnetic field in an ideal cavity with an oscillating boundary is considered in the resonance long-time limit. The rates of photon creation from the vacuum and thermal states are evaluated. The squeezing coefficients for the field modes are found, as well as the backward reaction of the field on the vibrating wall.

  8. Stochastic resonance and coherence resonance in groundwater-dependent plant ecosystems.

    PubMed

    Borgogno, Fabio; D'Odorico, Paolo; Laio, Francesco; Ridolfi, Luca

    2012-01-21

    Several studies have shown that non-linear deterministic dynamical systems forced by external random components can give rise to unexpectedly regular temporal behaviors. Stochastic resonance and coherence resonance, the two best known processes of this type, have been studied in a number of physical and chemical systems. Here, we explore their possible occurrence in the dynamics of groundwater-dependent plant ecosystems. To this end, we develop two eco-hydrological models, which allow us to demonstrate that stochastic and coherence resonance may emerge in the dynamics of phreatophyte vegetation, depending on their deterministic properties and the intensity of external stochastic drivers.

  9. Optical Helmholtz resonators

    NASA Astrophysics Data System (ADS)

    Chevalier, Paul; Bouchon, Patrick; Haïdar, Riad; Pardo, Fabrice

    2014-08-01

    Helmholtz resonators are widely used acoustic components able to select a single frequency. Here, based on an analogy between acoustics and electromagnetism wave equations, we present an electromagnetic 2D Helmholtz resonator made of a metallic slit-box structure. At the resonance, the light is funneled in the λ/800 apertures, and is subsequently absorbed in the cavity. As in acoustics, there is no higher order of resonance, which is an appealing feature for applications such as photodetection or thermal emission. Eventually, we demonstrate that the slit is of capacitive nature while the box behaves inductively. We derive an analytical formula for the resonance wavelength, which does not rely on wave propagation and therefore does not depend on the permittivity of the material filling the box. Besides, in contrast with half-wavelength resonators, the resonance wavelength can be engineered by both the slit aspect ratio and the box area.

  10. Magnetic resonance energy and topological resonance energy.

    PubMed

    Aihara, Jun-Ichi

    2016-04-28

    Ring-current diamagnetism of a polycyclic π-system is closely associated with thermodynamic stability due to the individual circuits. Magnetic resonance energy (MRE), derived from the ring-current diamagnetic susceptibility, was explored in conjunction with graph-theoretically defined topological resonance energy (TRE). For many aromatic molecules, MRE is highly correlative with TRE with a correlation coefficient of 0.996. For all π-systems studied, MRE has the same sign as TRE. The only trouble with MRE may be that some antiaromatic and non-alternant species exhibit unusually large MRE-to-TRE ratios. This kind of difficulty can in principle be overcome by prior geometry-optimisation or by changing spin multiplicity. Apart from the semi-empirical resonance-theory resonance energy, MRE is considered as the first aromatic stabilisation energy (ASE) defined without referring to any hypothetical polyene reference.

  11. Nucleon Resonance Physics

    NASA Astrophysics Data System (ADS)

    Burkert, Volker D.

    2016-10-01

    Recent results of meson photo-production at the existing electron machines with polarized real photon beams and the measurement of polarization observables of the final state baryons have provided high precision data that led to the discovery of new excited nucleon and Δ states using multi-channel partial wave analyses procedures. The internal structure of several prominent excited states has been revealed employing meson electroproduction processes. On the theoretical front, lattice QCD is now predicting the baryon spectrum with very similar characteristics as the constituent quark model, and continuum QCD, such as is represented in the Dyson-Schwinger equations approach and in light front relativistic quark models, describes the non-perturbative behavior of resonance excitations at photon virtuality of Q^2 > 1.5 GeV^2. In this talk I discuss the need to continue a vigorous program of nucleon spectroscopy and the study of the internal structure of excited states as a way to reveal the effective degrees of freedom underlying the excited states and their dependence on the distance scale probed.

  12. Resonant Versus Anti-Resonant Tunneling at Carbon Nanotube A-B-A Heterostructures

    NASA Technical Reports Server (NTRS)

    Mingo, N.; Yang, Liu; Han, Jie; Anantram, M. P.

    2001-01-01

    Narrow antiresonances going to zero transmission are found to occur for general (2n,0)(n,n)(2n,0) carbon nanotube heterostructures, whereas the complementary configuration, (n,n)(2n,0)(n,n), displays simple resonant tunneling behaviour. We compute examples for different cases, and give a simple explanation for the appearance of antiresonances in one case but not in the other. Conditions and ranges for the occurrence of these different behaviors are stated. The phenomenon of anti-resonant tunneling, which has passed unnoticed in previous studies of nanotube heterostructures, adds up to the rich set of behaviors available to nanotube based quantum effect devices.

  13. The Use and Evaluation of Scaffolding, Student Centered-Learning, Behaviorism, and Constructivism to Teach Nuclear Magnetic Resonance and IR Spectroscopy in a Two-Semester Organic Chemistry Course

    ERIC Educational Resources Information Center

    Livengood, Kimberly; Lewallen, Denver W.; Leatherman, Jennifer; Maxwell, Janet L.

    2012-01-01

    Since 2002, infrared spectroscopy (IR) and nuclear magnetic resonance (NMR) spectrometry have been introduced at the beginning of the first-semester organic chemistry lab course at this university. Starting in 2008, each individual student was given 20 unique homework problems that consisted of multiple-choice [superscript 1]H NMR and IR problems…

  14. Disorder-driven non-Fermi liquid behavior in single-crystalline Ce2Co0.8Si3.2.

    PubMed

    Szlawska, M; Kaczorowski, D

    2014-01-01

    A single crystal of the Ce-based ternary silicide Ce2Co0.8Si3.2, which crystallizes with a hexagonal AlB2-type related structure, was studied by means of magnetization, resistivity and heat capacity measurements. The compound was characterized as a Kondo paramagnet down to 0.4 K. Its low-temperature behavior is dominated by distinct non-Fermi liquid features, most likely arising due to structural disorder in the nonmagnetic-atom sublattice. PMID:24292411

  15. Quadrupole Induced Resonant Particle Transport

    NASA Astrophysics Data System (ADS)

    Gilson, Erik; Fajans, Joel

    1998-11-01

    We have performed experiments that explore the effects of a magnetic quadrupole field on a pure electron plasma confined in a Penning-Malmberg trap. A model that we have developed describes the shape of the plasma and shows that a certain class of resonant particles follows trajectories that take them out of the plasma. Even though the quadrupole field destroys the cylindrical symmetry of the system, our theory predicts that if the electrons are off resonance, then the lifetime of the plasma will not be greatly affected by the quadrupole field. Our preliminary experimental results show that the shape of the plasma and the plasma lifetime agree with our model. We are investigating the scaling of this behavior with various experimental parameters such as the plasma length, density, and strength of the quadrupole field. In addition to being an example of resonant particle transport, this effect may find practical applications in experiments that plan to use magnetic quadrupole neutral atom traps to confine anti-hydrogen created in double-well positron/anti-proton Penning-Malmberg traps. (ATHENA Collaboration.)

  16. Quadrupole Induced Resonant Particle Transport

    NASA Astrophysics Data System (ADS)

    Gilson, Erik; Fajans, Joel

    1999-11-01

    We have performed experiments that explore the effects of a magnetic quadrupole field on a pure electron plasma confined in a Malmberg-Penning trap. A model that we have developed describes the shape of the plasma and shows that a certain class of resonant particles follows trajectories that take them out of the plasma. Even though the quadrupole field destroys the cylindrical symmetry of the system, our theory predicts that if the electrons are off resonance, then the lifetime of the plasma will not be greatly affected by the quadrupole field. Our preliminary experimental results show that the shape of the plasma and the plasma lifetime agree with our model. We are investigating the scaling of this behavior with various experimental parameters such as the plasma length, density, and strength of the quadrupole field. In addition to being an example of resonant particle transport, this effect may find practical applications in experiments that plan to use magnetic quadrupole neutral atom traps to confine anti-hydrogen created in double-well positron/anti-proton Malmberg-Penning traps. (ATHENA Collaboration.)

  17. Emergent behavior in strongly correlated electron systems.

    PubMed

    Pines, David

    2016-09-01

    I describe early work on strongly correlated electron systems (SCES) from the perspective of a theoretical physicist who, while a participant in their reductionist top-down beginnings, is now part of the paradigm change to a bottom-up 'emergent' approach with its focus on using phenomenology to find the organizing principles responsible for their emergent behavior disclosed by experiment-and only then constructing microscopic models that incorporate these. After considering the organizing principles responsible for the emergence of plasmons, quasiparticles, and conventional superconductivity in SCES, I consider their application to three of SCES's sister systems, the helium liquids, nuclei, and the nuclear matter found in neutron stars. I note some recent applications of the random phase approximation and examine briefly the role that paradigm change is playing in two central problems in our field: understanding the emergence and subsequent behavior of heavy electrons in Kondo lattice materials; and finding the mechanism for the unconventional superconductivity found in heavy electron, organic, cuprate, and iron-based materials. PMID:27484183

  18. Emergent behavior in strongly correlated electron systems

    NASA Astrophysics Data System (ADS)

    Pines, David

    2016-09-01

    I describe early work on strongly correlated electron systems (SCES) from the perspective of a theoretical physicist who, while a participant in their reductionist top-down beginnings, is now part of the paradigm change to a bottom-up ‘emergent’ approach with its focus on using phenomenology to find the organizing principles responsible for their emergent behavior disclosed by experiment—and only then constructing microscopic models that incorporate these. After considering the organizing principles responsible for the emergence of plasmons, quasiparticles, and conventional superconductivity in SCES, I consider their application to three of SCES’s sister systems, the helium liquids, nuclei, and the nuclear matter found in neutron stars. I note some recent applications of the random phase approximation and examine briefly the role that paradigm change is playing in two central problems in our field: understanding the emergence and subsequent behavior of heavy electrons in Kondo lattice materials; and finding the mechanism for the unconventional superconductivity found in heavy electron, organic, cuprate, and iron-based materials.

  19. Excitonic surface lattice resonances

    NASA Astrophysics Data System (ADS)

    Humphrey, A. D.; Gentile, M. J.; Barnes, W. L.

    2016-08-01

    Electromagnetic resonances are important in controlling light at the nanoscale. The most studied such resonance is the surface plasmon resonance that is associated with metallic nanostructures. Here we explore an alternative resonance, the surface exciton-polariton resonance, one based on excitonic molecular materials. Our study is based on analytical and numerical modelling. We show that periodic arrays of suitable molecular nanoparticles may support surface lattice resonances that arise as a result of coherent interactions between the particles. Our results demonstrate that excitonic molecular materials are an interesting alternative to metals for nanophotonics; they offer the prospect of both fabrication based on supramolecular chemistry and optical functionality arising from the way the properties of such materials may be controlled with light.

  20. Shape resonance phenomena in CO following K-shell photoexcitation

    SciTech Connect

    Truesdale, C.M.; Southworth, S.H.; Kobrin, P.H.; Becker, U.; Lindle, D.W.; Kerkhoff, H.G.; Shirley, D.A.

    1983-04-25

    Electron cross sections and asymmetries following photoexcitation of the CO K shells were measured directly. Energy analysis of ejected electrons yielded cross sections exhibiting sigma shape resonances in the C(1s), C(KVV), and O(1s) channels, and a ..pi.. resonance in the C(KVV) channel, confirming earlier indirect measurements. Asymmetry measurements showed a sigma shape resonance in the C(1s) channel, in good agreement with the predictions of Dehmer and Dill. The C(KVV) ..pi.. resonance showed nearly isotropic behavior.

  1. Mechanical Resonances of Helically Coiled Carbon Nanowires

    NASA Astrophysics Data System (ADS)

    Saini, D.; Behlow, H.; Podila, R.; Dickel, D.; Pillai, B.; Skove, M. J.; Serkiz, S. M.; Rao, A. M.

    2014-07-01

    Despite their wide spread applications, the mechanical behavior of helically coiled structures has evaded an accurate understanding at any length scale (nano to macro) mainly due to their geometrical complexity. The advent of helically coiled micro/nanoscale structures in nano-robotics, nano-inductors, and impact protection coatings has necessitated the development of new methodologies for determining their shear and tensile properties. Accordingly, we developed a synergistic protocol which (i) integrates analytical, numerical (i.e., finite element using COMSOL®) and experimental (harmonic detection of resonance; HDR) methods to obtain an empirically validated closed form expression for the shear modulus and resonance frequency of a singly clamped helically coiled carbon nanowire (HCNW), and (ii) circumvents the need for solving 12th order differential equations. From the experimental standpoint, a visual detection of resonances (using in situ scanning electron microscopy) combined with HDR revealed intriguing non-planar resonance modes at much lower driving forces relative to those needed for linear carbon nanotube cantilevers. Interestingly, despite the presence of mechanical and geometrical nonlinearities in the HCNW resonance behavior the ratio of the first two transverse modes f2/f1 was found to be similar to the ratio predicted by the Euler-Bernoulli theorem for linear cantilevers.

  2. Mechanical Resonances of Helically Coiled Carbon Nanowires

    PubMed Central

    Saini, D.; Behlow, H.; Podila, R.; Dickel, D.; Pillai, B.; Skove, M. J.; Serkiz, S. M.; Rao, A. M.

    2014-01-01

    Despite their wide spread applications, the mechanical behavior of helically coiled structures has evaded an accurate understanding at any length scale (nano to macro) mainly due to their geometrical complexity. The advent of helically coiled micro/nanoscale structures in nano-robotics, nano-inductors, and impact protection coatings has necessitated the development of new methodologies for determining their shear and tensile properties. Accordingly, we developed a synergistic protocol which (i) integrates analytical, numerical (i.e., finite element using COMSOL®) and experimental (harmonic detection of resonance; HDR) methods to obtain an empirically validated closed form expression for the shear modulus and resonance frequency of a singly clamped helically coiled carbon nanowire (HCNW), and (ii) circumvents the need for solving 12th order differential equations. From the experimental standpoint, a visual detection of resonances (using in situ scanning electron microscopy) combined with HDR revealed intriguing non-planar resonance modes at much lower driving forces relative to those needed for linear carbon nanotube cantilevers. Interestingly, despite the presence of mechanical and geometrical nonlinearities in the HCNW resonance behavior the ratio of the first two transverse modes f2/f1 was found to be similar to the ratio predicted by the Euler-Bernoulli theorem for linear cantilevers. PMID:24986377

  3. Acoustic Levitator Maintains Resonance

    NASA Technical Reports Server (NTRS)

    Barmatz, M. B.; Gaspar, M. S.

    1986-01-01

    Transducer loading characteristics allow resonance tracked at high temperature. Acoustic-levitation chamber length automatically adjusted to maintain resonance at constant acoustic frequency as temperature changes. Developed for containerless processing of materials at high temperatures, system does not rely on microphones as resonance sensors, since microphones are difficult to fabricate for use at temperatures above 500 degrees C. Instead, system uses acoustic transducer itself as sensor.

  4. Large mode radius resonators

    NASA Technical Reports Server (NTRS)

    Harris, Michael R.

    1987-01-01

    Resonator configurations permitting operation with large mode radius while maintaining good transverse mode discrimination are considered. Stable resonators incorporating an intracavity telescope and unstable resonator geometries utilizing an output coupler with a Gaussian reflectivity profile are shown to enable large radius single mode laser operation. Results of heterodyne studies of pulsed CO2 lasers with large (11mm e sup-2 radius) fundamental mode sizes are presented demonstrating minimal frequency sweeping in accordance with the theory of laser-induced medium perturbations.

  5. Measuring Shell Resonances of Spherical Acoustic Resonators

    NASA Astrophysics Data System (ADS)

    Truong, D.; Sparasci, F.; Foltête, E.; Ouisse, M.; Pitre, L.

    2011-01-01

    Coupling between the gas and shell is a concern in the experiment used at LNE-CNAM to determine the Boltzmann constant k B by an acoustic method. As the walls of real resonators are not perfectly rigid, some perturbations occur in the frequency range of the acoustic resonances measured within helium gas contained in the cavity. As a contribution for a better understanding of this phenomenon, an experiment to measure the shell modes of the spherical resonators is in use in this laboratory. A work in progress to assess these modes using a hammer blow method together with modal analysis is reported here. The study is carried out with an air-filled, copper-walled, half-liter quasi-spherical resonator in the frequency range from 1 Hz to 20 kHz. Results show that the shell modes expand into multiple resonances of similar modal shape, including the "breathing" mode. The observations reported in other studies of shell perturbations at other frequencies than the breathing frequency are confirmed.

  6. On open electromagnetic resonators: relation between interferometers and resonators

    SciTech Connect

    Manenkov, Aleksandr A; Bykov, Vladimir P; Kuleshov, N V

    2010-05-26

    The physical difference between the concepts 'Fabry-Perot interferometer' and 'open resonator' is discussed. It is shown that the use of the term 'Fabry-Perot resonator' for open laser resonators is incorrect both from the historical viewpoint and from the viewpoint of the physical meaning of the processes occurring in these resonators. (laser beams and resonators)

  7. Fluid mechanical model of the Helmholtz resonator

    NASA Technical Reports Server (NTRS)

    Hersh, A. S.; Walker, B.

    1977-01-01

    A semi-empirical fluid mechanical model of the acoustic behavior of Helmholtz resonators is presented which predicts impedance as a function of the amplitude and frequency of the incident sound pressure field and resonator geometry. The model assumes that the particle velocity approaches the orifice in a spherical manner. The incident and cavity sound fields are connected by solving the governing oscillating mass and momentum conservation equations. The model is in agreement with the Rayleigh slug-mass model at low values of incident sound pressure level. At high values, resistance is predicted to be independent of frequency, proportional to the square root of the amplitude of the incident sound pressure field, and virtually independent of resonator geometry. Reactance is predicted to depend in a very complicated way upon resonator geometry, incident sound pressure level, and frequency. Nondimensional parameters are defined that divide resonator impedance into three categories corresponding to low, moderately low, and intense incident sound pressure amplitudes. The two-microphone method was used to measure the impedance of a variety of resonators. The data were used to refine and verify the model.

  8. Stochastic resonance in models of neuronal ensembles

    SciTech Connect

    Chialvo, D.R. Longtin, A.; Mueller-Gerkin, J.

    1997-02-01

    Two recently suggested mechanisms for the neuronal encoding of sensory information involving the effect of stochastic resonance with aperiodic time-varying inputs are considered. It is shown, using theoretical arguments and numerical simulations, that the nonmonotonic behavior with increasing noise of the correlation measures used for the so-called aperiodic stochastic resonance (ASR) scenario does not rely on the cooperative effect typical of stochastic resonance in bistable and excitable systems. Rather, ASR with slowly varying signals is more properly interpreted as linearization by noise. Consequently, the broadening of the {open_quotes}resonance curve{close_quotes} in the multineuron {ital stochastic resonance without tuning} scenario can also be explained by this linearization. Computation of the input-output correlation as a function of both signal frequency and noise for the model system further reveals conditions where noise-induced firing with aperiodic inputs will benefit from stochastic resonance rather than linearization by noise. Thus, our study clarifies the tuning requirements for the optimal transduction of subthreshold aperiodic signals. It also shows that a single deterministic neuron can perform as well as a network when biased into a suprathreshold regime. Finally, we show that the inclusion of a refractory period in the spike-detection scheme produces a better correlation between instantaneous firing rate and input signal. {copyright} {ital 1997} {ital The American Physical Society}

  9. Modeling of dielectric elastomer as electromechanical resonator

    SciTech Connect

    Li, Bo Liu, Lei; Chen, Hualing; Jia, Shuhai; Zhang, Junshi; Li, Dichen

    2014-09-28

    Dielectric elastomers (DEs) feature nonlinear dynamics resulting from an electromechanical coupling. Under alternating voltage, the DE resonates with tunable performances. We present an analysis of the nonlinear dynamics of a DE as electromechanical resonator (DEER) configured as a pure shear actuator. A theoretical model is developed to characterize the complex performance under different boundary conditions. Physical mechanisms are presented and discussed. Chaotic behavior is also predicted, illustrating instabilities in the dynamics. The results provide a guide to the design and application of DEER in haptic devices.

  10. Modeling of dielectric elastomer as electromechanical resonator

    NASA Astrophysics Data System (ADS)

    Li, Bo; Zhang, Junshi; Liu, Lei; Chen, Hualing; Jia, Shuhai; Li, Dichen

    2014-09-01

    Dielectric elastomers (DEs) feature nonlinear dynamics resulting from an electromechanical coupling. Under alternating voltage, the DE resonates with tunable performances. We present an analysis of the nonlinear dynamics of a DE as electromechanical resonator (DEER) configured as a pure shear actuator. A theoretical model is developed to characterize the complex performance under different boundary conditions. Physical mechanisms are presented and discussed. Chaotic behavior is also predicted, illustrating instabilities in the dynamics. The results provide a guide to the design and application of DEER in haptic devices.

  11. Granular convection observed by magnetic resonance imaging

    SciTech Connect

    Ehrichs, E.E.; Jaeger, H.M.; Knight, J.B.; Nagel, S.R.; Karczmar, G.S.; Kuperman, V.Yu.

    1995-03-17

    Vibrations in a granular material can spontaneously produce convection rolls reminiscent of those seen in fluids. Magnetic resonance imaging provides a sensitive and noninvasive probe for the detection of these convection currents, which have otherwise been difficult to observe. A magnetic resonance imaging study of convection in a column of poppy seeds yielded data about the detailed shape of the convection rolls and the depth dependence of the convection velocity. The velocity was found to decrease exponentially with depth; a simple model for this behavior is presented here. 31 refs., 4 figs.

  12. HTS nonlinearities in microwave disk resonators

    NASA Astrophysics Data System (ADS)

    Collado, Carlos; Mateu, Jordi; Shaw, Timothy J.; O'Callaghan, Juan M.

    2002-08-01

    This article describes a procedure for the calculation of the intermodulation behavior of the TM0 1 0 mode in high temperature superconducting (HTS) disk resonators from a description of the local HTS nonlinearities. Successful cross-checks are performed by comparing the theoretical results with experimental measurements and simulations based on the multiport harmonic balance algorithm for a specific model of HTS nonlinearity. The application of this procedure to the determination of nonlinear material parameters from disk resonator measurements is illustrated and compared to theoretical predictions.

  13. Granular convection observed by magnetic resonance imaging

    NASA Astrophysics Data System (ADS)

    Ehrichs, E. E.; Jaeger, H. M.; Karczmar, Greg S.; Knight, James B.; Kuperman, Vadim Yu.; Nagel, Sidney R.

    1995-03-01

    Vibrations in a granular material can spontaneously produce convection rolls reminiscent of those seen in fluids. Magnetic resonance imaging provides a sensitive and noninvasive probe for the detection of these convection currents, which have otherwise been difficult to observe. A magnetic resonance imaging study of convection in a column of poppy seeds yielded data about the detailed shape of the convection rolls and the depth dependence of the convection velocity. The velocity was found to decrease exponentially with depth; a simple model for this behavior is presented here.

  14. Cardiovascular Magnetic Resonance Imaging

    NASA Astrophysics Data System (ADS)

    Pelc, Norbert

    2000-03-01

    Cardiovascular diseases are a major source of morbidity and mortality in the United States. Early detection of disease can often be used to improved outcomes, either through direct interventions (e.g. surgical corrections) or by causing the patient to modify his or her behavior (e.g. smoking cessation or dietary changes). Ideally, the detection process should be noninvasive (i.e. it should not be associated with significant risk). Magnetic Resonance Imaging (MRI) refers to the formation of images by localizing NMR signals, typically from protons in the body. As in other applications of NMR, a homogeneous static magnetic field ( ~0.5 to 4 T) is used to create ``longitudinal" magnetization. A magnetic field rotating at the Larmor frequency (proportional to the static field) excites spins, converting longitudinal magnetization to ``transverse" magnetization and generating a signal. Localization is performed using pulsed gradients in the static field. MRI can produce images of 2-D slices, 3-D volumes, time-resolved images of pseudo-periodic phenomena such as heart function, and even real-time imaging. It is also possible to acquire spatially localized NMR spectra. MRI has a number of advantages, but perhaps the most fundamental is the richness of the contrast mechanisms. Tissues can be differentiated by differences in proton density, NMR properties, and even flow or motion. We also have the ability to introduce substances that alter NMR signals. These contrast agents can be used to enhance vascular structures and measure perfusion. Cardiovascular MRI allows the reliable diagnosis of important conditions. It is possible to image the blood vessel tree, quantitate flow and perfusion, and image cardiac contraction. Fundamentally, the power of MRI as a diagnostic tool stems from the richness of the contrast mechanisms and the flexibility in control of imaging parameters.

  15. Analysis of plasmon resonances on a metal particle

    NASA Astrophysics Data System (ADS)

    Bakhti, Saïd; Destouches, Nathalie; Tishchenko, Alexandre V.

    2014-10-01

    An analytical representation of plasmon resonance modes of a metal particle is developed in the basis of the null-field method and its modal expansion of the particle optical response. This representation allows for the characterization of plasmon modes properties, as their spectral position, bandwidth, amplitude and local field enhancement. Moreover, the derivation of a phenomenological equation governing such resonances relates them to open resonator behavior. The resonance bandwidth corresponds to the plasmon life-time, whereas its amplitude is related to the coupling coefficient with the incident excitation. An efficient algorithm is used to compute and characterize the resonance parameters of silver spheroids as function of the particle geometry. The normal modes present on spheres are split into different azimuthal resonant modes in the case of spheroids, with amplitude depending on the incident polarization and position dependent on the particle aspect ratio.

  16. Optical Haroche and Hanle resonances

    NASA Astrophysics Data System (ADS)

    Ruyten, Wilhelmus M.

    1990-07-01

    It is shown that Haroche and Hanle resonances, known from magnetic resonance, should be observable in an optical resonance experiment in which a narrowband, phase-modulated laser resonantly excites a two-level system. The narrow Haroche resonances should allow the first observation of an optical Bloch-Siegert shift, and may find applications in modulation spectroscopy.

  17. The Concept of Resonance

    ERIC Educational Resources Information Center

    Truhlar, Donald G.

    2007-01-01

    A general example of a delocalization system associated with a higher energy than the localized one, which suggests that it is wrong to consider delocalization as equivalent to resonance stabilization, is presented. The meaning of resonance energy as it appears in valence bond theory is described as the lowering of the calculated ground-state…

  18. Ballistic spin resonance.

    PubMed

    Frolov, S M; Lüscher, S; Yu, W; Ren, Y; Folk, J A; Wegscheider, W

    2009-04-16

    The phenomenon of spin resonance has had far-reaching influence since its discovery 70 years ago. Electron spin resonance driven by high-frequency magnetic fields has enhanced our understanding of quantum mechanics, and finds application in fields as diverse as medicine and quantum information. Spin resonance can also be induced by high-frequency electric fields in materials with a spin-orbit interaction; the oscillation of the electrons creates a momentum-dependent effective magnetic field acting on the electron spin. Here we report electron spin resonance due to a spin-orbit interaction that does not require external driving fields. The effect, which we term ballistic spin resonance, is driven by the free motion of electrons that bounce at frequencies of tens of gigahertz in micrometre-scale channels of a two-dimensional electron gas. This is a frequency range that is experimentally challenging to access in spin resonance, and especially difficult on a chip. The resonance is manifest in electrical measurements of pure spin currents-we see a strong suppression of spin relaxation length when the oscillating spin-orbit field is in resonance with spin precession in a static magnetic field. These findings illustrate how the spin-orbit interaction can be harnessed for spin manipulation in a spintronic circuit, and point the way to gate-tunable coherent spin rotations in ballistic nanostructures without external alternating current fields. PMID:19370029

  19. The resonator handbook

    NASA Technical Reports Server (NTRS)

    Cook, Jerry D.; Zhou, Shiliang

    1993-01-01

    The purpose of this work is to extend resonator theory into the region in which the planar mirror is quite small. Results of the theoretical description are then extended to resonator design and experimental arrangements as discussed in further sections of this work. Finally, a discussion of dielectric measurements for small samples is included as a specific application of this work.

  20. Multi-orbital non-crossing approximation from maximally localized Wannier functions: the Kondo signature of copper phthalocyanine on Ag(100).

    PubMed

    Korytár, Richard; Lorente, Nicolás

    2011-09-01

    We have developed a multi-orbital approach to compute the electronic structure of a quantum impurity using the non-crossing approximation. The calculation starts with a mean-field evaluation of the system's electronic structure using a standard quantum chemistry code; here we use density functional theory (DFT). We transformed the one-electron structure into an impurity Hamiltonian by using maximally localized Wannier functions. Hence, we have developed a method to study the Kondo effect in systems based on an initial one-electron calculation. We have applied our methodology to a copper phthalocyanine molecule chemisorbed on Ag(100), and we have described its spectral function for three different cases where the molecule presents a single spin or two spins with ferro- and anti-ferromagnetic exchange couplings. We find that the use of broken-symmetry mean-field theories such as Kohn-Sham DFT cannot deal with the complexity of the spin of open-shell molecules on metal surfaces and extra modeling is needed.