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Sample records for laser field time-dependent

  1. Correlated multielectron systems in strong laser fields: A multiconfiguration time-dependent Hartree-Fock approach

    SciTech Connect

    Caillat, J.; Scrinzi, A.; Koch, O.; Kreuzer, W.

    2005-01-01

    The multiconfiguration time-dependent Hartree-Fock approach for the description of correlated few-electron dynamics in the presence of strong laser fields is introduced and a comprehensive description of the method is given. Total ionization and electron spectra for the ground and first excited ionic channels are calculated for one-dimensional model systems with up to six active electrons. Strong correlation effects are found in the shape of photoelectron peaks and the dependence of ionization on molecule size.

  2. Simulation of electron dynamics subject to intense laser fields using a time-dependent Volkov basis

    NASA Astrophysics Data System (ADS)

    Covington, Cody; Kidd, Daniel; Gilmer, Justin; Varga, Kálmán

    2017-01-01

    We present various intense laser-driven electron dynamics simulations performed using a Volkov basis set and compare results with other popular choices of basis. The Volkov basis is comprised of plane waves modified by a time-dependent phase factor, allowing for improved accuracy over other representations such as a real-space grid or plane-wave basis. Alternatively, this advantage may be realized by being afforded significantly larger time-step sizes in wave-function propagation techniques. Comparisons of the Volkov basis set to other popular bases have been carried out for model one-dimensional finite and periodic systems as well as three-dimensional systems using time-dependent density functional theory, and the efficiency and accuracy of the Volkov approach have been demonstrated.

  3. Laser-assisted field evaporation of metal oxides: A time-dependent density functional theory study

    NASA Astrophysics Data System (ADS)

    Xia, Yu; Li, Zhibing

    2016-11-01

    To understand laser-assisted field evaporation of semiconductors and insulators at the microscopic level, we study the time evolution of the electronic and atomic structure of a MgO cluster in high electrostatic fields subjected to strong laser pulses. We find that the critical laser intensity for evaporation decreases linearly as the electrostatic field strength increases. The optical absorption enhancement in high electrostatic field is confirmed by the redshift of the optical absorption spectra, the reduction of the energy gap, and the increase of the absorption cross section.

  4. Information entropy of a time-dependent three-level trapped ion interacting with a laser field

    NASA Astrophysics Data System (ADS)

    Abdel-Aty, Mahmoud

    2005-10-01

    Trapped and laser-cooled ions are increasingly used for a variety of modern high-precision experiments, frequency standard applications and quantum information processing. Therefore, in this communication we present a comprehensive analysis of the pattern of information entropy arising in the time evolution of an ion interacting with a laser field. A general analytic approach is proposed for a three-level trapped-ion system in the presence of the time-dependent couplings. By working out an exact analytic solution, we conclusively analyse the general properties of the von Neumann entropy and quantum information entropy. It is shown that the information entropy is affected strongly by the time-dependent coupling and exhibits long time periodic oscillations. This feature attributed to the fact that in the time-dependent region Rabi oscillation is time dependent. Using parameters corresponding to a specific three-level ionic system, a single beryllium ion in a RF-(Paul) trap, we obtain illustrative examples of some novel aspects of this system in the dynamical evolution. Our results establish an explicit relation between the exact information entropy and the entanglement between the multi-level ion and the laser field. We show that different nonclassical effects arise in the dynamics of the ionic population inversion, depending on the initial states of the vibrational motion/field and on the values of Lamb-Dicke parameter η.

  5. Precision treatment of single and double multiphoton ionization of He atoms by strong laser fields: Time-dependent generalized pseudospectral method in internal coordinates

    NASA Astrophysics Data System (ADS)

    Telnov, Dmitry A.; Heslar, John; Chu, Shih-I.

    2012-06-01

    We have developed a new computational method for accurate and efficient numerical solution of the time-dependent Schr"odinger equation for two-electron atoms. Our approach is full-dimensional and makes use of the internal coordinates of the electrons in the plane defined by the electrons and the nucleus (r1, r2, and θ12) as well as Euler angles which determine the orientation of the plane in space. The internal coordinates can be optimally discretized by means of the generalized pseudospectral method while the Euler angles appear through the basis set functions with the definite total angular momentum and its projections. The results of the single and double ionization of the helium atom by strong 800 nm laser fields will be presented. The accurate time-dependent electron density obtained can be used for testing and improvement of various approximate exchange-correlation functionals of the time-dependent density functional theory.

  6. Vacuum radiation induced by time dependent electric field

    NASA Astrophysics Data System (ADS)

    Zhang, Bo; Zhang, Zhi-meng; Hong, Wei; He, Shu-Kai; Teng, Jian; Gu, Yu-qiu

    2017-04-01

    Many predictions of new phenomena given by strong field quantum electrodynamics (SFQED) will be tested on next generation multi-petawatt laser facilities in the near future. These new phenomena are basis to understand physics in extremely strong electromagnetic fields therefore have attracted wide research interest. Here we discuss a new SFQED phenomenon that is named as vacuum radiation. In vacuum radiation, a virtual electron loop obtain energy from time dependent external electric field and radiate an entangled photon pair. Features of vacuum radiation in a locally time dependent electric field including spectrum, characteristic temperature, production rate and power are given.

  7. Recent development of self-interaction-free time-dependent density-functional theory for nonperturbative treatment of atomic and molecular multiphoton processes in intense laser fields.

    PubMed

    Chu, Shih-I

    2005-08-08

    In this paper, we present a short account of some recent developments of self-interaction-free density-functional theory (DFT) and time-dependent density-functional theory (TDDFT) for accurate and efficient treatment of the electronic structure, and time-dependent quantum dynamics of many-electron atomic and molecular systems. The conventional DFT calculations using approximate and explicit exchange-correlation energy functional contain spurious self-interaction energy and improper long-range asymptotic potential, preventing reliable treatment of the excited, resonance, and continuum states. We survey some recent developments of DFT/TDDFT with optimized effective potential (OEP) and self-interaction correction (SIC) for both atomic and molecular systems for overcoming some of the above mentioned difficulties. These DFT (TDDFT)/OEP-SIC approaches allow the use of orbital-independent single-particle local potential which is self-interaction free. In addition we discuss several numerical techniques recently developed for efficient and high-precision treatment of the self-interaction-free DFT/TDDFT equations. The usefulness of these procedures is illustrated by a few case studies of atomic, molecular, and condensed matter processes of current interests, including (a) autoionizing resonances, (b) relativistic OEP-SIC treatment of atomic structure (Z=2-106), (c) shell-filling electronic structure in quantum dots, (d) atomic and molecular processes in intense laser fields, including multiphoton ionization, and very-high-order harmonic generation, etc. For the time-dependent processes, an alternative Floquet formulation of TDDFT is introduced for time-independent treatment of multiphoton processes in intense periodic or quasiperiodic fields. We conclude this paper with some open questions and perspectives of TDDFT.

  8. Heating liquid dielectrics by time dependent fields

    NASA Astrophysics Data System (ADS)

    Khalife, A.; Pathak, U.; Richert, R.

    2011-10-01

    Steady state and time-resolved dielectric relaxation experiments are performed at high fields on viscous glycerol and the effects of energy absorption from the electric field are studied. Time resolution is obtained by a sinusoidal field whose amplitude is switched from a low to a high level and by recording voltage and current traces with an oscilloscope during this transition. Based on their distinct time and frequency dependences, three sources of modifying the dynamics and dielectric loss via an increase in the effective temperature can be distinguished: electrode temperature, real sample temperature, and configurational temperatures of the modes that absorbed the energy. Isothermal conditions that are desired for focusing on the configurational temperature changes (as in dielectric hole burning and related techniques) are maintained only for very thin samples and for moderate power levels. For high frequencies, say ν > 1 MHz, changes of the real temperature will exceed the effects of configurational temperatures in the case of macroscopic samples. Regarding microwave chemistry, heating via cell phone use, and related situations in which materials are subject to fields involving frequencies beyond the MHz regime, we conclude that changes in the configurational (or fictive) temperatures remain negligible compared with the increase of the real temperature. This simplifies the assessment of how time dependent electric fields modify the properties of materials.

  9. Stable and efficient momentum-space solutions of the time-dependent Schrödinger equation for one-dimensional atoms in strong laser fields

    SciTech Connect

    Shvetsov-Shilovski, N.I. Räsänen, E.

    2014-12-15

    One-dimensional model systems have a particular role in strong-field physics when gaining physical insight by computing data over a large range of parameters, or when performing numerous time propagations within, e.g., optimal control theory. Here we derive a scheme that removes a singularity in the one-dimensional Schrödinger equation in momentum space for a particle in the commonly used soft-core Coulomb potential. By using this scheme we develop two numerical approaches to the time-dependent Schrödinger equation in momentum space. The first approach employs the expansion of the momentum-space wave function over the eigenstates of the field-free Hamiltonian, and it is shown to be more efficient for laser parameters usual in strong field physics. The second approach employs the Crank–Nicolson scheme or the method of lines for time-propagation. The both methods are readily applicable for large-scale numerical simulations in one-dimensional model systems.

  10. Time dependent theory for random lasers

    PubMed

    Jiang; Soukoulis

    2000-07-03

    A model to simulate the phenomenon of random lasing is presented. It couples Maxwell's equations with the rate equations of electronic population in a disordered system. Finite difference time domain methods are used to obtain the field pattern and the spectra of localized lasing modes inside the system. A critical pumping rate P(c)(r) exists for the appearance of the lasing peaks. The number of lasing modes increases with the pumping rate and the length of the system. There is a lasing mode repulsion. This property leads to a saturation of the number of modes for a given size system and a relation between the localization length xi and average mode length L(m).

  11. Time-dependent numerical simulation of vertical cavity lasers

    SciTech Connect

    Thode, L.E.; Csanak, G.; So, L.L.; Kwan, T.J.T.; Campbell, M.

    1994-12-31

    To simulate vertical cavity surface emitting lasers (VCSELs), the authors are developing a three-dimensional, time-dependent field-gain model with absorption in bulk dielectric regions and gain in quantum well regions. Since the laser linewidth is narrow, the bulk absorption coefficient is assumed to be independent of frequency with a value determined by the material and the lattice temperature. In contrast, the frequency-dependent gain regions must be solved consistently in the time domain. Treatment of frequency-dependent media in a finite-difference time-domain code is computationally intensive. However, because the volume of the quantum well regions is small relative to the volume of the multilayer dielectric (MLD) mirror regions, the computational overhead is reasonable. A key issue is the calculation of the fields in the MLD mirror regions. Although computationally intensive, good agreement has been obtained between simulation results and matrix equation solutions for the reflection coefficient, transmission coefficient, and bandwidth of MLD mirrors. The authors discuss the development and testing of the two-dimensional field-gain model. This field-gain model will be integrated with a carrier transport model to form the self-consistent laser code, VCSEL.

  12. Description of molecular dynamics in intense laser fields by the time-dependent adiabatic state approach: application to simultaneous two-bond dissociation of CO2 and its control.

    PubMed

    Sato, Yukio; Kono, Hirohiko; Koseki, Shiro; Fujimura, Yuichi

    2003-07-02

    We theoretically investigated the dynamics of structural deformations of CO(2) and its cations in near-infrared intense laser fields (approximately 10(15) W cm(-2)) by using the time-dependent adiabatic state approach. To obtain "field-following" adiabatic potentials for nuclear dynamics, the electronic Hamiltonian including the interaction with the instantaneous laser electric field is diagonalized by the multiconfiguration self-consistent-field molecular orbital method. In the CO(2) and CO(2+) stages, ionization occurs before the field intensity becomes high enough to deform the molecule. In the CO(2)(2+) stage, simultaneous symmetric two-bond stretching occurs as well as one-bond stretching. Two-bond stretching is induced by an intense field in the lowest time-dependent adiabatic state |1> of CO(2)(2+), and this two-bond stretching is followed by the occurrence of a large-amplitude bending motion mainly in the second-lowest adiabatic state |2> nonadiabatically created at large internuclear distances by the field from |1>. It is concluded that the experimentally observed stretched and bent structure of CO(2)(3+) just before Coulomb explosions originates from the structural deformation of CO(2)(2+). We also show in this report that the concept of "optical-cycle-averaged potential" is useful for designing schemes to control molecular (reaction) dynamics, such as dissociation dynamics of CO(2), in intense fields. The present approach is simple but has wide applicability for analysis and prediction of electronic and nuclear dynamics of polyatomic molecules in intense laser fields.

  13. Time-dependent restricted-active-space self-consistent-field theory for laser-driven many-electron dynamics. II. Extended formulation and numerical analysis

    NASA Astrophysics Data System (ADS)

    Miyagi, Haruhide; Madsen, Lars Bojer

    2014-06-01

    The time-dependent restricted-active-space self-consistent-field (TD-RASSCF) method is formulated based on the TD variational principle. The SCF based TD orbitals contributing to the expansion of the wave function are classified into three groups, between which orbital excitations are considered with the RAS scheme. In analogy with the configuration-interaction singles (CIS), singles-and-doubles (CISD), and singles-doubles-and-triples (CISDT) methods in quantum chemistry, the TD-RASSCF-S, -SD, and -SDT methods are introduced as extensions of the TD-RASSCF-doubles (-D) method [Phys. Rev. A 87, 062511 (2013), 10.1103/PhysRevA.87.062511]. Based on an analysis of the numerical cost and test calculations for one-dimensional (1D) models of atomic helium, beryllium, and carbon, it is shown that the TD-RASSCF-S and -D methods are computationally feasible for systems with many electrons and more accurate than the TD Hartree-Fock (TDHF) and TDCIS methods. In addition to the discussion of methodology, an analysis of electron dynamics in the high-order harmonic generation (HHG) process is presented. For the 1D beryllium atom, a state-resolved analysis of the HHG spectrum based on the time-independent HF orbitals shows that while only single-orbital excitations are needed in the region below the cutoff, single- and double-orbital excitations are essential beyond, where accordingly the single-active-electron (SAE) approximation and the TDCIS method break down. On the other hand, the TD-RASSCF-S and -D methods accurately describe the multiorbital excitation processes throughout the entire region of the HHG spectrum. For the 1D carbon atom, our calculations show that multiorbital excitations are essential in the HHG process even below the cutoff. Hence, in this test system a very accurate treatment of electron correlation is required. The TD-RASSCF-S and -D approaches meet this demand, while the SAE approximation and the TDCIS method are inadequate.

  14. Time dependent electromagnetic fields and 4-dimensional Stokes' theorem

    NASA Astrophysics Data System (ADS)

    Andosca, Ryan; Singleton, Douglas

    2016-11-01

    Stokes' theorem is central to many aspects of physics—electromagnetism, the Aharonov-Bohm effect, and Wilson loops to name a few. However, the pedagogical examples and research work almost exclusively focus on situations where the fields are time-independent so that one need only deal with purely spatial line integrals (e.g., ∮ A . d x ) and purely spatial area integrals (e.g., ∫ ( ∇ × A ) . d a = ∫ B . d a ). Here, we address this gap by giving some explicit examples of how Stokes' theorem plays out with time-dependent fields in a full 4-dimensional spacetime context. We also discuss some unusual features of Stokes' theorem with time-dependent fields related to gauge transformations and non-simply connected topology.

  15. Time-dependent neutron and photon dose-field analysis

    NASA Astrophysics Data System (ADS)

    Wooten, Hasani Omar

    2005-11-01

    A unique tool is developed that allows the user to model physical representations of complicated glovebox facilities in two dimensions and determine neutral-particle flux and ambient dose-equivalent fields throughout that geometry. The code Pandemonium, originally designed to determine flux and dose rates only, has been improved to include realistic glovebox geometries, time-dependent source and detector positions, time-dependent shielding thickness calculations, time-integrated doses, a representative criticality accident scenario based on time-dependent reactor kinetics, and more rigorous photon treatment. The photon model has been significantly enhanced by expanding the energy range to 10 MeV to include fission photons, and by including a set of new buildup factors, the result of an extensive study into the previously unknown "purely-angular effect" on photon buildup. Purely-angular photon buildup factors are determined using discrete ordinates and coupled electron-photon cross sections to account for coherent and incoherent scattering and secondary photon effects of bremsstrahlung and florescence. Improvements to Pandemonium result in significant modeling capabilities for processing facilities using intense neutron and photon sources, and the code obtains comparable results to Monte Carlo calculations but within a fraction of the time required to run such codes as MCNPX.

  16. Subcycle dynamics of high-order-harmonic generation of He atoms excited by attosecond pulses and driven by near-infrared laser fields: A self-interaction-free time-dependent density-functional-theory approach

    NASA Astrophysics Data System (ADS)

    Heslar, John; Telnov, Dmitry A.; Chu, Shih-I.

    2014-05-01

    In the framework of the self-interaction-free time-dependent density-functional theory, we have performed three-dimensional (3D) ab initio calculations of He atoms in near-infrared (NIR) laser fields subject to excitation by a single extreme ultraviolet (XUV) attosecond pulse (SAP). We have explored the dynamical behavior of the subcycle high harmonic generation (HHG) for transitions from the excited states to the ground state and found oscillation structures with respect to the time delay between the SAP and NIR fields. The oscillatory pattern in the photon emission spectra has a period of ˜1.3 fs which is half of the NIR laser optical cycle, similar to that recently measured in the experiments on transient absorption of He [M. Chini et al., Sci. Rep. 3, 1105 (2013), 10.1038/srep01105]. We present the photon emission spectra from 1s2p, 1s3p, 1s4p, 1s5p, and 1s6p excited states as functions of the time delay. We explore the subcycle Stark shift phenomenon in NIR fields and its influence on the photon emission process. Our analysis reveals several interesting features of the subcycle HHG dynamics and we identify the mechanisms responsible for the observed peak splitting in the photon emission spectra.

  17. Time-dependent scalar fields as candidates for dark matter

    NASA Astrophysics Data System (ADS)

    Malakolkalami, B.; Mahmoodzadeh, A.

    2016-11-01

    In this paper, we study some properties of what is called the oscillaton, a spherically symmetric object made of a real time-dependent scalar field. Using an exponential scalar potential instead of a quadratic one discussed in previous works, as a new choice, we investigate the oscillaton properties with this potential. Solving the differential equation system resulting from the Einstein-Klein-Gordon equations reveals the importance of the oscillatons as candidates for dark matter. Meanwhile, a simplification called the stationary limit procedure is also carried out.

  18. Time-Dependent Neutron and Photon Dose-Field Analysis

    SciTech Connect

    Wooten, Hasani Omar

    2005-08-01

    A unique tool is developed that allows the user to model physical representations of complicated glovebox facilities in two dimensions and determine neutral-particle flux and ambient dose-equivalent fields throughout that geometry. The Pandemonium code, originally designed to determine flux and dose-rates only, is improved to include realistic glovebox geometries, time-dependent source and detector positions, time-dependent shielding thickness calculations, time-integrated doses, a representative criticality accident scenario based on time-dependent reactor kinetics, and more rigorous photon treatment. A primary benefit of this work has been an extensive analysis and improvement of the photon model that is not limited to the application described in this thesis. The photon model has been extended in energy range to 10 MeV to include photons from fission and new photon buildup factors have been included that account for the effects of photon buildup at slant-path thicknesses as a function of angle, where the mean free path thickness has been preserved. The overall system of codes is user-friendly and it is directly applicable to facilities such as the plutonium facility at Los Alamos National Laboratory, where high-intensity neutron and photon emitters are regularly used. The codes may be used to determine a priori doses for given work scenarios in an effort to supply dose information to process models which will in turn assist decision makers on ensuring as low as reasonably achievable (ALARA) compliance. In addition, coupling the computational results of these tools with the process model visualization tools will help to increase worker safety and radiological safety awareness.

  19. Extended time-dependent mean-field approximation

    SciTech Connect

    Portes, D.A. Jr. |; Kodama, T.; de Toledo Piza, A.F.

    1996-09-01

    The time-dependent mean-field approximation for two dynamically coupled subsystems is extended to include correlation effects between the subsystems, allowing for decorrelation processes to develop in the reduced density matrices. The extended scheme is formulated in terms of the truncation to {ital M} terms of the Schmidt decomposition of the full density matrix. This {ital M} natural orbitals truncation scheme is compared to the exact numerical solution for a system of two coupled anharmonic oscillators in a factorized initial state. It is found that the approximation {ital M}=3 gives a good approximation to the exact results over several characteristic times of the system. {copyright} {ital 1996 The American Physical Society.}

  20. Stokes phenomenon and schwinger vacuum pair production in time-dependent laser pulses.

    PubMed

    Dumlu, Cesim K; Dunne, Gerald V

    2010-06-25

    Particle production due to external fields (electric, chromoelectric, or gravitational) requires evolving an initial state through an interaction with a time-dependent background, with the rate being computed from a Bogoliubov transformation between the in and out vacua. When the background fields have temporal profiles with substructure, a semiclassical analysis of this problem confronts the full subtlety of the Stokes phenomenon: WKB solutions are only local, while the production rate requires global information. We give a simple quantitative explanation of the recently computed [Phys. Rev. Lett. 102, 150404 (2009)10.1103/PhysRevLett.102.150404] oscillatory momentum spectrum of e^{+}e^{-} pairs produced from vacuum subjected to a time-dependent electric field with subcycle laser pulse structure. This approach also explains naturally why for spinor and scalar QED these oscillations are out of phase.

  1. Stokes Phenomenon and Schwinger Vacuum Pair Production in Time-Dependent Laser Pulses

    SciTech Connect

    Dumlu, Cesim K.; Dunne, Gerald V.

    2010-06-25

    Particle production due to external fields (electric, chromoelectric, or gravitational) requires evolving an initial state through an interaction with a time-dependent background, with the rate being computed from a Bogoliubov transformation between the in and out vacua. When the background fields have temporal profiles with substructure, a semiclassical analysis of this problem confronts the full subtlety of the Stokes phenomenon: WKB solutions are only local, while the production rate requires global information. We give a simple quantitative explanation of the recently computed [Phys. Rev. Lett. 102, 150404 (2009)] oscillatory momentum spectrum of e{sup +}e{sup -} pairs produced from vacuum subjected to a time-dependent electric field with subcycle laser pulse structure. This approach also explains naturally why for spinor and scalar QED these oscillations are out of phase.

  2. Time-dependent intensity and phase measurements of ultrashort laser pulses as short as 10 fs

    SciTech Connect

    DeLong, K.W.; Fittinghoff, D.N.; Ladera, C.L.; Trebino, R.; Taft, G.; Rundquist, A.; Murnane, M.M.; Kapteyn, H.C.; Christov, I.P.

    1995-05-01

    Frequency-Resolved Optical Gating (FROG) measures the time-dependent intensity and phase of an ultrashort laser pulse. Using FROG, we have tested theories for the operation of sub{minus}10 fs laser oscillators.

  3. Time-dependent QED model for high-order harmonic generation in ultrashort intense laser pulses

    NASA Astrophysics Data System (ADS)

    Hu, Huayu; Yuan, Jianmin

    2008-12-01

    To advance the QED approach and exploit more details of the high-order harmonic generation (HHG) of atoms and molecules in intense ultrashort laser fields, a QED model for HHG is developed in a time-dependent framework and a multimode-laser setup. By introduction of the classical-field-dressed quantized Volkov states, an analytical expression to calculate HHG for hydrogenlike atoms and ions in an ultrashort intense laser pulse is obtained. This formula provides a simple intuitive interpretation of the mechanism in which the electron is first ionized to the classical-field-dressed quantized Volkov states, and then falls back to the ground state to emit the harmonic photon. Calculations using this formalism demonstrate a good agreement with recent semiclassical computations. The limiting of the existing QED models, which are successful in providing alternative perspectives on the HHG beyond semiclassical treatments, to the time-independent framework and the single-mode laser have been removed to take into account the laser pulse’s length and its shape. Possible extensive applications of this QED approach as well as its potential usefulness for research in various interesting fields are also discussed. The long-wavelength approximation and strong-field approximation are involved in the development of the formalism.

  4. Delay time dependence of thermal effect of combined pulse laser machining

    NASA Astrophysics Data System (ADS)

    Yuan, Boshi; Jin, Guangyong; Ma, Yao; Zhang, Wei

    2016-10-01

    The research focused on the effect of delay time in combined pulse laser machining on the material temperature field. Aiming at the parameter optimization of pulse laser machining aluminum alloy, the combined pulse laser model based on heat conduction equation was introduced. And the finite element analysis software, COMSOL Multiphysics, was also utilized in the research. Without considering the phase transition process of aluminum alloy, the results of the numerical simulation was shown in this paper. By the simulation study of aluminum alloy's irradiation with combined pulse, the effect of the change in delay time of combined pulse on the temperature field of the aluminum alloy and simultaneously the quantized results under the specific laser spot conditions were obtained. Based on the results, several conclusions could be reached, the delay time could affect the rule of temperature changing with time. The reasonable delay time controlling would help improving the efficiency. In addition, when the condition of the laser pulse energy density is constant, the optimal delay time depends on pulse sequence.

  5. Time-dependent quantum chemistry of laser driven many-electron molecules.

    PubMed

    Nguyen-Dang, Thanh-Tung; Couture-Bienvenue, Étienne; Viau-Trudel, Jérémy; Sainjon, Amaury

    2014-12-28

    A Time-Dependent Configuration Interaction approach using multiple Feshbach partitionings, corresponding to multiple ionization stages of a laser-driven molecule, has recently been proposed [T.-T. Nguyen-Dang and J. Viau-Trudel, J. Chem. Phys. 139, 244102 (2013)]. To complete this development toward a fully ab-initio method for the calculation of time-dependent electronic wavefunctions of an N-electron molecule, we describe how tools of multiconfiguration quantum chemistry such as the management of the configuration expansion space using Graphical Unitary Group Approach concepts can be profitably adapted to the new context, that of time-resolved electronic dynamics, as opposed to stationary electronic structure. The method is applied to calculate the detailed, sub-cycle electronic dynamics of BeH2, treated in a 3-21G bound-orbital basis augmented by a set of orthogonalized plane-waves representing continuum-type orbitals, including its ionization under an intense λ = 800 nm or λ = 80 nm continuous-wave laser field. The dynamics is strongly non-linear at the field-intensity considered (I ≃ 10(15) W/cm(2)), featuring important ionization of an inner-shell electron and strong post-ionization bound-electron dynamics.

  6. Time-dependent quantum chemistry of laser driven many-electron molecules

    SciTech Connect

    Nguyen-Dang, Thanh-Tung; Couture-Bienvenue, Étienne; Viau-Trudel, Jérémy; Sainjon, Amaury

    2014-12-28

    A Time-Dependent Configuration Interaction approach using multiple Feshbach partitionings, corresponding to multiple ionization stages of a laser-driven molecule, has recently been proposed [T.-T. Nguyen-Dang and J. Viau-Trudel, J. Chem. Phys. 139, 244102 (2013)]. To complete this development toward a fully ab-initio method for the calculation of time-dependent electronic wavefunctions of an N-electron molecule, we describe how tools of multiconfiguration quantum chemistry such as the management of the configuration expansion space using Graphical Unitary Group Approach concepts can be profitably adapted to the new context, that of time-resolved electronic dynamics, as opposed to stationary electronic structure. The method is applied to calculate the detailed, sub-cycle electronic dynamics of BeH{sub 2}, treated in a 3–21G bound-orbital basis augmented by a set of orthogonalized plane-waves representing continuum-type orbitals, including its ionization under an intense λ = 800 nm or λ = 80 nm continuous-wave laser field. The dynamics is strongly non-linear at the field-intensity considered (I ≃ 10{sup 15} W/cm{sup 2}), featuring important ionization of an inner-shell electron and strong post-ionization bound-electron dynamics.

  7. Developments in deep brain stimulation using time dependent magnetic fields

    SciTech Connect

    Crowther, L.J.; Nlebedim, I.C.; Jiles, D.C.

    2012-03-07

    The effect of head model complexity upon the strength of field in different brain regions for transcranial magnetic stimulation (TMS) has been investigated. Experimental measurements were used to verify the validity of magnetic field calculations and induced electric field calculations for three 3D human head models of varying complexity. Results show the inability for simplified head models to accurately determine the site of high fields that lead to neuronal stimulation and highlight the necessity for realistic head modeling for TMS applications.

  8. Developments in deep brain stimulation using time dependent magnetic fields

    NASA Astrophysics Data System (ADS)

    Crowther, L. J.; Nlebedim, I. C.; Jiles, D. C.

    2012-04-01

    The effect of head model complexity upon the strength of field in different brain regions for transcranial magnetic stimulation (TMS) has been investigated. Experimental measurements were used to verify the validity of magnetic field calculations and induced electric field calculations for three 3D human head models of varying complexity. Results show the inability for simplified head models to accurately determine the site of high fields that lead to neuronal stimulation and highlight the necessity for realistic head modeling for TMS applications.

  9. Quantum Diffusion Monte Carlo Method for strong field time dependent problems

    NASA Astrophysics Data System (ADS)

    Kalinski, Matt

    2006-05-01

    We formulate the Quantum Diffusion Quantum Monte Carlo (QDMC) method for the solution of the time-dependent Schr"odinger equation for atoms in strong laser fields. Unlike for the normal diffusion Monte Carlo the wave function is represented by walkers with two kinds or colors which solve two coupled and nonlinear diffusion equations. Those diffusion equations are coupled by the potentials similar to those introduced by Shay which must be added to Schr"odingers equation to obtain classical dynamics equivalent to the quantum mechanics [1]. The potentials are calculated semi-analytically similarly to smoothing methods of smooth particle electrodynamics (SPD) with Gaussian smoothing kernels. We apply this method to strong field two electron ionization of Helium. We calculate two electron double ionization rate in full six-dimensional configuration space quantum mechanically. Comparison with classical mechanics and the low dimensional grid models is also provided. 1cm [1] D. Shay, Phys. Rev A 13, 2261 (1976)

  10. Field quantization and squeezed states generation in resonators with time-dependent parameters

    NASA Technical Reports Server (NTRS)

    Dodonov, V. V.; Klimov, A. B.; Nikonov, D. E.

    1992-01-01

    The problem of electromagnetic field quantization is usually considered in textbooks under the assumption that the field occupies some empty box. The case when a nonuniform time-dependent dielectric medium is confined in some space region with time-dependent boundaries is studied. The basis of the subsequent consideration is the system of Maxwell's equations in linear passive time-dependent dielectric and magnetic medium without sources.

  11. Extended gyrokinetic field theory for time-dependent magnetic confinement fields

    NASA Astrophysics Data System (ADS)

    Sugama, H.; Watanabe, T.-H.; Nunami, M.

    2014-01-01

    A gyrokinetic system of equations for turbulent toroidal plasmas in time-dependent axisymmetric background magnetic fields is derived from the variational principle. Besides governing equations for gyrocenter distribution functions and turbulent electromagnetic fields, the conditions which self-consistently determine the background magnetic fields varying on a transport time scale are obtained by using the Lagrangian, which includes the constraint on the background fields. Conservation laws for energy and toroidal angular momentum of the whole system in the time-dependent background magnetic fields are naturally derived by applying Noether's theorem. It is shown that the ensemble-averaged transport equations of particles, energy, and toroidal momentum given in the present work agree with the results from the conventional recursive formulation with the WKB representation except that collisional effects are disregarded here.

  12. Extended gyrokinetic field theory for time-dependent magnetic confinement fields

    SciTech Connect

    Sugama, H.; Watanabe, T.-H.; Nunami, M.

    2014-01-15

    A gyrokinetic system of equations for turbulent toroidal plasmas in time-dependent axisymmetric background magnetic fields is derived from the variational principle. Besides governing equations for gyrocenter distribution functions and turbulent electromagnetic fields, the conditions which self-consistently determine the background magnetic fields varying on a transport time scale are obtained by using the Lagrangian, which includes the constraint on the background fields. Conservation laws for energy and toroidal angular momentum of the whole system in the time-dependent background magnetic fields are naturally derived by applying Noether's theorem. It is shown that the ensemble-averaged transport equations of particles, energy, and toroidal momentum given in the present work agree with the results from the conventional recursive formulation with the WKB representation except that collisional effects are disregarded here.

  13. Non-Markovian Brownian motion in a magnetic field and time-dependent force fields

    NASA Astrophysics Data System (ADS)

    Hidalgo-Gonzalez, J. C.; Jiménez-Aquino, J. I.; Romero-Bastida, M.

    2016-11-01

    This work focuses on the derivation of the velocity and phase-space generalized Fokker-Planck equations for a Brownian charged particle embedded in a memory thermal bath and under the action of force fields: a constant magnetic field and arbitrary time-dependent force fields. To achieve the aforementioned goal we use a Gaussian but non-Markovian generalized Langevin equation with an arbitrary friction memory kernel. In a similar way, the generalized diffusion equation in the zero inertia limit is also derived. Additionally we show, in the absence of the time-dependent external forces, that, if the fluctuation-dissipation relation of the second kind is valid, then the generalized Langevin dynamics associated with the charged particle reaches a stationary state in the large-time limit. The consistency of our theoretical results is also verified when they are compared with those derived in the absence of the force fields and in the Markovian case.

  14. Second quantized scalar QED in homogeneous time-dependent electromagnetic fields

    SciTech Connect

    Kim, Sang Pyo

    2014-12-15

    We formulate the second quantization of a charged scalar field in homogeneous, time-dependent electromagnetic fields, in which the Hamiltonian is an infinite system of decoupled, time-dependent oscillators for electric fields, but it is another infinite system of coupled, time-dependent oscillators for magnetic fields. We then employ the quantum invariant method to find various quantum states for the charged field. For time-dependent electric fields, a pair of quantum invariant operators for each oscillator with the given momentum plays the role of the time-dependent annihilation and the creation operators, constructs the exact quantum states, and gives the vacuum persistence amplitude as well as the pair-production rate. We also find the quantum invariants for the coupled oscillators for the charged field in time-dependent magnetic fields and advance a perturbation method when the magnetic fields change adiabatically. Finally, the quantum state and the pair production are discussed when a time-dependent electric field is present in parallel to the magnetic field.

  15. Theory of time-dependent intense-field collisional resonance fluorescence

    NASA Technical Reports Server (NTRS)

    Kleiber, P. D.; Cooper, J.; Burnett, K.; Kunasz, C. V.; Raymer, M. G.

    1983-01-01

    The time-dependent theory of Courtens and Szoke (1977) is generalized using the approach of Burnett et al. (1982) to derive time-dependent spectral intensities of resonance fluorescence from atoms driven by a pulsed laser in the presence of collisions. These results are valid both for laser detunings inside and outside the usual impact region of the spectrum, including Zeeman degeneracy effects. This theory is applied to a simple but important example (J = 0 to J = 1) to obtain quantitative predictions for the observable scattered-light spectrum which can be directly compared with recent experiments.

  16. Simulating Time-Dependent Energy Transfer Between Crossed Laser Beams in an Expanding Plasma

    SciTech Connect

    Hittinger, J F; Dorr, M R; Berger, R L; Williams, E A

    2004-10-11

    A coupled mode system is derived to investigate a three-wave parametric instability leading to energy transfer between co-propagating laser beams crossing in a plasma flow. The model includes beams of finite width refracting in a prescribed transverse plasma flow with spatial and temporal gradients in velocity and density. The resulting paraxial light equations are discretized spatially with a Crank-Nicholson-type scheme, and these algebraic constraints are nonlinearly coupled with ordinary differential equations in time that describe the ion acoustic response. The entire nonlinear differential-algebraic system is solved using an adaptive, backward-differencing method coupled with Newton's method. A numerical study is conducted in two dimensions that compares the intensity gain of the fully time-dependent coupled mode system with the gain computed under the further assumption of a strongly-damped ion acoustic response. The results demonstrate a time-dependent gain suppression when the beam diameter is commensurate with the velocity gradient scale length. The gain suppression is shown to depend on time-dependent beam refraction and is interpreted as a time-dependent frequency shift.

  17. Time dependence of fast electron beam divergence in ultraintense laser-plasma interactions.

    PubMed

    Akli, K U; Storm, M J; McMahon, M; Jiang, S; Ovchinnikov, V; Schumacher, D W; Freeman, R R; Dyer, G; Ditmire, T

    2012-08-01

    We report on the measurement and computer simulation of the divergence of fast electrons generated in an ultraintense laser-plasma interaction (LPI) and the subsequent propagation in a nonrefluxing target. We show that, at Iλ(2) of 10(20) Wcm(-2)μm(2), the time-integrated electron beam full divergence angle is (60±5)°. However, our time-resolved 2D particle-in-cell simulations show the initial beam divergence to be much smaller (≤30°). Our simulations show the divergence to monotonically increase with time, reaching a final value of (68±7)° after the passage of the laser pulse, consistent with the experimental time-integrated measurements. By revealing the time-dependent nature of the LPI, we find that a substantial fraction of the laser energy (~7%) is transported up to 100 μm with a divergence of 32°.

  18. Time-dependent study of a black-hole laser in a flowing atomic condensate

    NASA Astrophysics Data System (ADS)

    de Nova, J. R. M.; Finazzi, S.; Carusotto, I.

    2016-10-01

    We numerically study the temporal evolution of a black-hole laser configuration displaying a pair of black- and white-hole horizons in a flowing atomic condensate. This configuration is initially prepared starting from a homogeneous flow via a suitable space-dependent change of the interaction constant and the evolution is then followed up to long times. Depending on the values of the system parameters, the system typically either converges to the lowest-energy solution by evaporating away the horizons or displays a continuous and periodic coherent emission of solitons. By making a physical comparison with optical laser devices, we identify the latter regime of continuous emission of solitons as the proper black-hole laser effect.

  19. Time-dependent 3-D modelling of laser surface heating for the hardening of metallic materials

    NASA Astrophysics Data System (ADS)

    Colombo, V.; Mentrelli, A.; Trombetti, T.

    2003-12-01

    A numerical code for the time-dependent three-dimensional modelling of the laser surface heating for the hardening of metallic materials has been developed by the authors. The temperature-dependence of the thermal properties of the material (stainless steel) is taken into account in the frame of a heating process that doesn’t lead to material melting or evaporation. Calculations have been carried out for various dimensions of the parallelepiped-shaped and of the square-shaped spot of the laser beam, as well as for different scanning velocity and for different levels of the laser source power. Various patterns of the laser spot path have also been studied, including a single-pass hardening pattern, a double-pass hardening pattern with and without overlapping, multiple discontinuous and continuous hardening patterns and spiral hardening patterns. The presented results show how the proposed model can be usefully employed in the prediction of the time-evolution of temperature distribution which arises in the workpiece as a consequence of the laser-workpiece interaction under operating conditions typically encountered in industrial applications of the laser hardening process.

  20. Time-dependent wettability of nano-patterned surfaces fabricated by femtosecond laser with high efficiency

    NASA Astrophysics Data System (ADS)

    Zhang, Yingchuan; Zou, Guisheng; Liu, Lei; Zhao, Yue; Liang, Qiong; Wu, Aiping; Zhou, Y. Norman

    2016-12-01

    High efficient fabrication of nanoscale surface structure has been achieved by line focusing a low repetition (1 kHz) femtosecond laser using a cylindrical lens. The results showed that this cylindrical lens increased fabrication rate by 10 times compared with a spherical lens. Both periodic ripple and random nanoparticle covered surface structures were obtained by optimizing the defocus distance and scanning speed. Strong time-dependent water contact angle (CA) was found in both laser patterned Cu and Ni surfaces. The random nanoparticle covered surface was superhydrophilic (around 1°) immediately after laser processing, but increased to ∼25° in the first day after exposed in air. The CA of periodic ripple surface showed a more obvious time dependency, in which a significant CA increasing (50° for Cu and 100° for Ni) was observed. The surface chemical analysis showed that absorption of hydrophobic functional groups changed the surface from the Wenzel state wetting to the Cassie state wetting, which was responsiblefor the hydrophilic to hydrophobic transition.

  1. Hydrodynamics of Exploding Foil X-Ray Lasers with Time-Dependent Ionization Effect

    NASA Astrophysics Data System (ADS)

    Wang, Yu; Su, Dandan; Li, Yingjun

    2016-12-01

    A simple modified model is presented based on R. A. London's self-similarity model on time-independent ionization hydrodynamics of exploding foil X-ray lasers. In our model, the time-dependent ionization effect is under consideration and the average ion charge depends on the temperature. Then we obtain the new scaling laws for temperature, scale length and electron density, which have better agreement with experimental results. supported by National Natural Science Foundation of China (Nos. 11574390, 11374360, 41472130) and the National Basic Research Program of China (No. 2013CBA01504)

  2. Motion of magnetospheric particle clouds in a time-dependent electric field model

    NASA Technical Reports Server (NTRS)

    Roederer, J. G.; Hones, E. H., Jr.

    1974-01-01

    A computer code has been developed to study quantitatively the drift motion of magnetospheric particles in a time-dependent electric field. These calculations were applied to the case of proton and electron injections from the plasma sheet during substorms; the model predictions were checked against observations on board the geosynchronous satellite ATS 5 by DeForest and McIlwain (1971). It was found that it is possible to simulate the observed proton spectrograms with an adequate choice of a time-dependent electric field model. The resulting kinematics is physically quite simple and in its gross features does not depend too strongly on the particular fine structure of the model.

  3. Angle-dependent strong-field molecular ionization rates with tuned range-separated time-dependent density functional theory

    NASA Astrophysics Data System (ADS)

    Sissay, Adonay; Abanador, Paul; Mauger, François; Gaarde, Mette; Schafer, Kenneth J.; Lopata, Kenneth

    2016-09-01

    Strong-field ionization and the resulting electronic dynamics are important for a range of processes such as high harmonic generation, photodamage, charge resonance enhanced ionization, and ionization-triggered charge migration. Modeling ionization dynamics in molecular systems from first-principles can be challenging due to the large spatial extent of the wavefunction which stresses the accuracy of basis sets, and the intense fields which require non-perturbative time-dependent electronic structure methods. In this paper, we develop a time-dependent density functional theory approach which uses a Gaussian-type orbital (GTO) basis set to capture strong-field ionization rates and dynamics in atoms and small molecules. This involves propagating the electronic density matrix in time with a time-dependent laser potential and a spatial non-Hermitian complex absorbing potential which is projected onto an atom-centered basis set to remove ionized charge from the simulation. For the density functional theory (DFT) functional we use a tuned range-separated functional LC-PBE*, which has the correct asymptotic 1/r form of the potential and a reduced delocalization error compared to traditional DFT functionals. Ionization rates are computed for hydrogen, molecular nitrogen, and iodoacetylene under various field frequencies, intensities, and polarizations (angle-dependent ionization), and the results are shown to quantitatively agree with time-dependent Schrödinger equation and strong-field approximation calculations. This tuned DFT with GTO method opens the door to predictive all-electron time-dependent density functional theory simulations of ionization and ionization-triggered dynamics in molecular systems using tuned range-separated hybrid functionals.

  4. Applying Boundary Conditions Using a Time-Dependent Lagrangian for Modeling Laser-Plasma Interactions

    NASA Astrophysics Data System (ADS)

    Reyes, Jonathan; Shadwick, B. A.

    2016-10-01

    Modeling the evolution of a short, intense laser pulse propagating through an underdense plasma is of particular interest in the physics of laser-plasma interactions. Numerical models are typically created by first discretizing the equations of motion and then imposing boundary conditions. Using the variational principle of Chen and Sudan, we spatially discretize the Lagrangian density to obtain discrete equations of motion and a discrete energy conservation law which is exactly satisfied regardless of the spatial grid resolution. Modifying the derived equations of motion (e.g., enforcing boundary conditions) generally ruins energy conservation. However, time-dependent terms can be added to the Lagrangian which force the equations of motion to have the desired boundary conditions. Although some foresight is needed to choose these time-dependent terms, this approach provides a mechanism for energy to exit the closed system while allowing the conservation law to account for the loss. An appropriate time discretization scheme is selected based on stability analysis and resolution requirements. We present results using this variational approach in a co-moving coordinate system and compare such results to those using traditional second-order methods. This work was supported by the U. S. Department of Energy under Contract No. DE-SC0008382 and by the National Science Foundation under Contract No. PHY- 1104683.

  5. Ultrafast strong-field photoelectron emission from biased metal surfaces: exact solution to time-dependent Schrödinger Equation.

    PubMed

    Zhang, Peng; Lau, Y Y

    2016-01-28

    Laser-driven ultrafast electron emission offers the possibility of manipulation and control of coherent electron motion in ultrashort spatiotemporal scales. Here, an analytical solution is constructed for the highly nonlinear electron emission from a dc biased metal surface illuminated by a single frequency laser, by solving the time-dependent Schrödinger equation exactly. The solution is valid for arbitrary combinations of dc electric field, laser electric field, laser frequency, metal work function and Fermi level. Various emission mechanisms, such as multiphoton absorption or emission, optical or dc field emission, are all included in this single formulation. The transition between different emission processes is analyzed in detail. The time-dependent emission current reveals that intense current modulation may be possible even with a low intensity laser, by merely increasing the applied dc bias. The results provide insights into the electron pulse generation and manipulation for many novel applications based on ultrafast laser-induced electron emission.

  6. On use of time-dependent microwave fields to increase an FEL oscillator efficiency

    SciTech Connect

    Saldin, E.L.; Schneidmiller, E.A.; Yurkov, M.V.

    1995-12-31

    Various schemes of a high efficiency FEL oscillator with time-dependent accelerating (or decelerating) microwave field in interaction region are proposed. All the, schemes are based on standard accelerating structure and undulator technology. Feasibility of the proposed schemes is confirmed by results of numerical simulations. Realistic examples of FEL oscillators of infrared and visible wavelength ranges with efficiency about 20 % are presented.

  7. Lie algebraic approach to the time-dependent quantum general harmonic oscillator and the bi-dimensional charged particle in time-dependent electromagnetic fields

    SciTech Connect

    Ibarra-Sierra, V.G.; Sandoval-Santana, J.C.; Cardoso, J.L.; Kunold, A.

    2015-11-15

    We discuss the one-dimensional, time-dependent general quadratic Hamiltonian and the bi-dimensional charged particle in time-dependent electromagnetic fields through the Lie algebraic approach. Such method consists in finding a set of generators that form a closed Lie algebra in terms of which it is possible to express a quantum Hamiltonian and therefore the evolution operator. The evolution operator is then the starting point to obtain the propagator as well as the explicit form of the Heisenberg picture position and momentum operators. First, the set of generators forming a closed Lie algebra is identified for the general quadratic Hamiltonian. This algebra is later extended to study the Hamiltonian of a charged particle in electromagnetic fields exploiting the similarities between the terms of these two Hamiltonians. These results are applied to the solution of five different examples: the linear potential which is used to introduce the Lie algebraic method, a radio frequency ion trap, a Kanai–Caldirola-like forced harmonic oscillator, a charged particle in a time dependent magnetic field, and a charged particle in constant magnetic field and oscillating electric field. In particular we present exact analytical expressions that are fitting for the study of a rotating quadrupole field ion trap and magneto-transport in two-dimensional semiconductor heterostructures illuminated by microwave radiation. In these examples we show that this powerful method is suitable to treat quadratic Hamiltonians with time dependent coefficients quite efficiently yielding closed analytical expressions for the propagator and the Heisenberg picture position and momentum operators. -- Highlights: •We deal with the general quadratic Hamiltonian and a particle in electromagnetic fields. •The evolution operator is worked out through the Lie algebraic approach. •We also obtain the propagator and Heisenberg picture position and momentum operators. •Analytical expressions for a

  8. Comment on 'Wave functions of a time-dependent harmonic oscillator in a static magnetic field'

    SciTech Connect

    Maamache, M.; Bounames, A.; Ferkous, N.

    2006-01-15

    We show that the procedure used by Ferreira et al. [Phys. Rev. A 66, 024103 (2002)] is not correct for the following reasons: (i) the invariant I(t) they derived does not satisfy the Liouville-Von Neuman equation. (ii) They found that the eigenvalues of I(t) are time dependent which should not be the case according to the Lewis-Riesenfeld theory. We give a correct procedure to find the solution of the system they considered, i.e., the Schroedinger equation for a two-dimensional harmonic oscillator with time-dependent mass and frequency in the presence of a static magnetic field.

  9. Wave function for dissipative harmonically confined electrons in a time-dependent electric field

    NASA Astrophysics Data System (ADS)

    Lai, Meng-Yun; Pan, Xiao-Yin; Li, Yu-Qi

    2016-07-01

    We investigate the many-body wave function of a dissipative system of interacting particles confined by a harmonic potential and perturbed by a time-dependent spatially homogeneous electric field. Applying the method of Yu and Sun (1994), it is found that the wave function is comprised of a phase factor times the solution to the unperturbed time-dependent (TD) Schrödinger equation with the latter being translated by a time-dependent value that satisfies the classical damped driven equation of motion, plus an addition fluctuation term due to the Brownian motion. The wave function reduces to that of the Harmonic Potential Theorem (HPT) wave function in the absence of the dissipation. An example of application of the results derived is also given.

  10. A time-dependent vector field topology based on streak surfaces.

    PubMed

    Uffinger, Markus; Sadlo, Filip; Ertl, Thomas

    2013-03-01

    It was shown recently how the 2D vector field topology concept, directly applicable to stationary vector fields only, can be generalized to time-dependent vector fields by replacing the role of stream lines by streak lines. The present paper extends this concept to 3D vector fields. In traditional 3D vector field topology separatrices can be obtained by integrating stream lines from 0D seeds corresponding to critical points. We show that in our new concept, in contrast, 1D seeding constructs are required for computing streak-based separatrices. In analogy to the 2D generalization we show that invariant manifolds can be obtained by seeding streak surfaces along distinguished path surfaces emanating from intersection curves between codimension-1 ridges in the forward and reverse finite-time Lyapunov exponent (FTLE) fields. These path surfaces represent a time-dependent generalization of critical points and convey further structure in time-dependent topology of vector fields. Compared to the traditional approach based on FTLE ridges, the resulting streak manifolds ease the analysis of Lagrangian coherent structures (LCS) with respect to visual quality and computational cost, especially when time series of LCS are computed. We exemplify validity and utility of the new approach using both synthetic examples and computational fluid dynamics results.

  11. Theoretical description of the mixed-field orientation of asymmetric-top molecules: A time-dependent study

    NASA Astrophysics Data System (ADS)

    Omiste, Juan J.; González-Férez, Rosario

    2016-12-01

    We present a theoretical study of the mixed-field-orientation of asymmetric-top molecules in tilted static electric field and nonresonant linearly polarized laser pulse by solving the time-dependent Schrödinger equation. Within this framework, we compute the mixed-field orientation of a state-selected molecular beam of benzonitrile (C7H5N ) and compare with the experimental observations [J. L. Hansen et al., Phys. Rev. A 83, 023406 (2011), 10.1103/PhysRevA.83.023406] and with our previous time-independent descriptions [J. J. Omiste et al., Phys. Chem. Chem. Phys. 13, 18815 (2011), 10.1039/c1cp21195a]. For an excited rotational state, we investigate the field-dressed dynamics for several field configurations as those used in the mixed-field experiments. The nonadiabatic phenomena and their consequences on the rotational dynamics are analyzed in detail.

  12. Landau levels of scalar QED in time-dependent magnetic fields

    SciTech Connect

    Kim, Sang Pyo

    2014-05-15

    The Landau levels of scalar QED undergo continuous transitions under a homogeneous, time-dependent magnetic field. We analytically formulate the Klein–Gordon equation for a charged spinless scalar as a Cauchy initial value problem in the two-component first order formalism and then put forth a measure that classifies the quantum motions into the adiabatic change, the nonadiabatic change, and the sudden change. We find the exact quantum motion and calculate the pair-production rate when the magnetic field suddenly changes as a step function. -- Highlights: •We study the Landau levels of scalar QED in time-dependent magnetic fields. •Instantaneous Landau levels make continuous transitions but keep parity. •The Klein–Gordon equation is expressed in the two-component first order formalism. •A measure is advanced that characterizes the quantum motions into three categories. •A suddenly changing magnetic field produces pairs of charged scalars from vacuum.

  13. Time-dependent Liouville density functional theory for laser-induced ultrafast demagnetization in ferromagnets

    NASA Astrophysics Data System (ADS)

    Zhang, Guoping; Bai, Yihua; George, Thomas F.

    Abstract: The traditional time-dependent density functional theory is very powerful to simulate the dynamic process, but is very time consuming. When it was first used to understand laser-induced ultrafast demagnetization in ferromagnets, the results were disappointing, with the laser amplitude at least three orders of magnitude larger than the experimental one to achieve the similar spin reduction. We develop a new theory within the density functional theory (DFT) for laser-induced ultrafast demagnetization in ferromagnets. We first solve the Liouville equation in the time domain and then feed the excited state density into the DFT code, so the dynamics proceeds on the excited and constraint potential surface. We test this for several magnetic systems and find a significantly larger demagnetization than the static approach, but is still smaller than the experimental finding. Both the local density approximation and the generalized gradient approximation fail. Our finding strongly suggests that a new functional must be developed. As a first test, we introduce a spin power scaling method. Some primitive results will be presented. This work was solely supported by the U.S. Department of Energy under Contract No. DE-FG02-06ER46304. The research used resources of the National Energy Research Scientific Computing Center.

  14. Time-dependent theoretical description of molecular autoionization produced by femtosecond xuv laser pulses

    SciTech Connect

    Sanz-Vicario, Jose Luis; Bachau, Henri; Martin, Fernando

    2006-03-15

    We present a nonperturbative time-dependent theoretical method to study H{sub 2} ionization with femtosecond laser pulses when the photon energy is large enough to populate the Q{sub 1} (25-28 eV) and Q{sub 2} (30-37 eV) doubly excited autoionizing states. We have investigated the role of these states in dissociative ionization of H{sub 2} and analyzed, in the time domain, the onset of the resonant peaks appearing in the proton kinetic energy distribution. Their dependence on photon frequency and pulse duration is also analyzed. The results are compared with available experimental data and with previous theoretical results obtained within a stationary perturbative approach. The method allows us as well to obtain dissociation yields corresponding to the decay of doubly excited states into two H atoms. The calculated H(n=2) yields are in good agreement with the experimental ones.

  15. The development of the time dependence of the nuclear EMP electric field

    SciTech Connect

    Eng, C

    2009-10-30

    The nuclear electromagnetic pulse (EMP) electric field calculated with the legacy code CHAP is compared with the field given by an integral solution of Maxwell's equations, also known as the Jefimenko equation, to aid our current understanding on the factors that affect the time dependence of the EMP. For a fair comparison the CHAP current density is used as a source in the Jefimenko equation. At first, the comparison is simplified by neglecting the conduction current and replacing the standard atmosphere with a constant density air slab. The simplicity of the resultant current density aids in determining the factors that affect the rise, peak and tail of the EMP electric field versus time. The three dimensional nature of the radiating source, i.e. sources off the line-of-sight, and the time dependence of the derivative of the current density with respect to time are found to play significant roles in shaping the EMP electric field time dependence. These results are found to hold even when the conduction current and the standard atmosphere are properly accounted for. Comparison of the CHAP electric field with the Jefimenko electric field offers a direct validation of the high-frequency/outgoing wave approximation.

  16. Spin interference in Rashba metal ring in a time-dependent magnetic field

    NASA Astrophysics Data System (ADS)

    Chen, Ji; Abdul Jalil, Mansoor Bin; Ghee Tan, Seng

    2013-05-01

    We investigate spin transport in a metal square ring with a strong Rashba spin orbit coupling (RSOC) effect, in the presence of a time-dependent magnetic field. We show that RSOC can be regarded as a spin-dependent gauge field which imparts a spin-dependent geometric phase (Aharonov-Casher phase) to conduction electrons in the ring. Combining the Aharonov-Bohm phase due to the time-dependent magnetic field with the able Aharonov-Casher phase due to RSOC, we are able to construct a spin interference condition, which modulates spin transport in the ring. The spin transport in the system is calculated via the tight-binding non-equilibrium Green's function formalism. Based on our transport calculations, we proposed a potential application of the Rashba square ring system as an alternating spin current generator.

  17. Unitarity Bounds and RG Flows in Time Dependent Quantum Field Theory

    SciTech Connect

    Dong, Xi; Horn, Bart; Silverstein, Eva; Torroba, Gonzalo; /Stanford U., ITP /Stanford U., Phys. Dept. /SLAC

    2012-04-05

    We generalize unitarity bounds on operator dimensions in conformal field theory to field theories with spacetime dependent couplings. Below the energy scale of spacetime variation of the couplings, their evolution can strongly affect the physics, effectively shifting the infrared operator scaling and unitarity bounds determined from correlation functions in the theory. We analyze this explicitly for large-N double-trace flows, and connect these to UV complete field theories. One motivating class of examples comes from our previous work on FRW holography, where this effect explains the range of flavors allowed in the dual, time dependent, field theory.

  18. Tuning of barrier crossing time of a particle by time dependent magnetic field.

    PubMed

    Baura, Alendu; Ray, Somrita; Bag, Bidhan Chandra

    2013-06-28

    We have studied the effect of time dependent magnetic field on the barrier crossing dynamics of a charged particle. An interplay of the magnetic field induced electric field and the applied field reveals several interesting features. For slowly oscillating field the barrier crossing rate increases remarkably particularly at large amplitude of the field. For appreciably large frequency a generically distinct phenomenon appears by virtue of parametric resonance manifested in multiple peaks appearing in the variation of the mean first passage time as a function of the amplitude. The parametric resonance is more robust against the variation of amplitude of the oscillating field compared to the case of variation of frequency. The barrier crossing time of a particle can be tuned para-metrically by appropriate choice of amplitude and frequency of the oscillating magnetic field.

  19. Resolution-of-identity stochastic time-dependent configuration interaction for dissipative electron dynamics in strong fields.

    PubMed

    Klinkusch, Stefan; Tremblay, Jean Christophe

    2016-05-14

    In this contribution, we introduce a method for simulating dissipative, ultrafast many-electron dynamics in intense laser fields. The method is based on the norm-conserving stochastic unraveling of the dissipative Liouville-von Neumann equation in its Lindblad form. The N-electron wave functions sampling the density matrix are represented in the basis of singly excited configuration state functions. The interaction with an external laser field is treated variationally and the response of the electronic density is included to all orders in this basis. The coupling to an external environment is included via relaxation operators inducing transition between the configuration state functions. Single electron ionization is represented by irreversible transition operators from the ionizing states to an auxiliary continuum state. The method finds its efficiency in the representation of the operators in the interaction picture, where the resolution-of-identity is used to reduce the size of the Hamiltonian eigenstate basis. The zeroth-order eigenstates can be obtained either at the configuration interaction singles level or from a time-dependent density functional theory reference calculation. The latter offers an alternative to explicitly time-dependent density functional theory which has the advantage of remaining strictly valid for strong field excitations while improving the description of the correlation as compared to configuration interaction singles. The method is tested on a well-characterized toy system, the excitation of the low-lying charge transfer state in LiCN.

  20. Time-dependent density functional theory for strong-field ionization by circularly polarized pulses

    NASA Astrophysics Data System (ADS)

    Chirilă, Ciprian C.; Lein, Manfred

    2017-03-01

    By applying time-dependent density functional theory to a two-dimensional multielectron atom subject to strong circularly polarized light pulses, we confirm that the ionization of p orbitals with defined angular momentum depends on the sense of rotation of the applied field. A simple ad-hoc modification of the adiabatic local-density exchange-correlation functional is proposed to remedy its unphysical behavior under orbital depletion.

  1. Representation independent algorithms for molecular response calculations in time-dependent self-consistent field theories

    SciTech Connect

    Tretiak, Sergei

    2008-01-01

    Four different numerical algorithms suitable for a linear scaling implementation of time-dependent Hartree-Fock and Kohn-Sham self-consistent field theories are examined. We compare the performance of modified Lanczos, Arooldi, Davidson, and Rayleigh quotient iterative procedures to solve the random-phase approximation (RPA) (non-Hermitian) and Tamm-Dancoff approximation (TDA) (Hermitian) eigenvalue equations in the molecular orbital-free framework. Semiempirical Hamiltonian models are used to numerically benchmark algorithms for the computation of excited states of realistic molecular systems (conjugated polymers and carbon nanotubes). Convergence behavior and stability are tested with respect to a numerical noise imposed to simulate linear scaling conditions. The results single out the most suitable procedures for linear scaling large-scale time-dependent perturbation theory calculations of electronic excitations.

  2. Representation independent algorithms for molecular response calculations in time-dependent self-consistent field theories

    NASA Astrophysics Data System (ADS)

    Tretiak, Sergei; Isborn, Christine M.; Niklasson, Anders M. N.; Challacombe, Matt

    2009-02-01

    Four different numerical algorithms suitable for a linear scaling implementation of time-dependent Hartree-Fock and Kohn-Sham self-consistent field theories are examined. We compare the performance of modified Lanczos, Arooldi, Davidson, and Rayleigh quotient iterative procedures to solve the random-phase approximation (RPA) (non-Hermitian) and Tamm-Dancoff approximation (TDA) (Hermitian) eigenvalue equations in the molecular orbital-free framework. Semiempirical Hamiltonian models are used to numerically benchmark algorithms for the computation of excited states of realistic molecular systems (conjugated polymers and carbon nanotubes). Convergence behavior and stability are tested with respect to a numerical noise imposed to simulate linear scaling conditions. The results single out the most suitable procedures for linear scaling large-scale time-dependent perturbation theory calculations of electronic excitations.

  3. Landau level transitions in doped graphene in a time dependent magnetic field

    NASA Astrophysics Data System (ADS)

    Ardenghi, J. S.; Bechthold, P.; Jasen, P.; Gonzalez, E.; Nagel, O.

    2013-10-01

    The aim of this work is to describe the Landau level transitions of Bloch electrons in doped graphene with an arbitrary time dependent magnetic field in the long wavelength approximation. In particular, transitions from the m Landau level to the m±1 and m±2 Landau levels are studied using the time dependent perturbation theory. Time intervals are computed in which transition probabilities tend to zero at a low order in the coupling constant. In particular, Landau level transitions are studied in the case of Bloch electrons traveling in the direction of the applied magnetic force and the results are compared with classical and revival periods of electrical current in graphene. Finally, current probabilities are computed for the n=0 and n=1 Landau levels showing expected oscillating behavior with modified cyclotron frequency.

  4. Modeling molecule-plasmon interactions using quantized radiation fields within time-dependent electronic structure theory

    SciTech Connect

    Nascimento, Daniel R.; DePrince, A. Eugene

    2015-12-07

    We present a combined cavity quantum electrodynamics/ab initio electronic structure approach for simulating plasmon-molecule interactions in the time domain. The simple Jaynes-Cummings-type model Hamiltonian typically utilized in such simulations is replaced with one in which the molecular component of the coupled system is treated in a fully ab initio way, resulting in a computationally efficient description of general plasmon-molecule interactions. Mutual polarization effects are easily incorporated within a standard ground-state Hartree-Fock computation, and time-dependent simulations carry the same formal computational scaling as real-time time-dependent Hartree-Fock theory. As a proof of principle, we apply this generalized method to the emergence of a Fano-like resonance in coupled molecule-plasmon systems; this feature is quite sensitive to the nanoparticle-molecule separation and the orientation of the molecule relative to the polarization of the external electric field.

  5. Dynamics of runaway tails with time-dependent sub-Dreicer dc fields in magnetized plasmas

    NASA Technical Reports Server (NTRS)

    Moghaddam-Taaheri, E.; Vlahos, L.

    1987-01-01

    The evolution of runaway tails driven by sub-Dreicer time-dependent dc fields in a magnetized plasma are studied numerically using a quasi-linear code based on the Ritz-Galerkin method and finite elements. It is found that the runaway tail maintained a negative slope during the dc field increase. Depending on the values of the dc electric field at t = 0 and the electron gyrofrequency to the plasma frequency ratio the runaway tail became unstable to the anomalous Doppler resonance or remained stable before the saturation of the dc field at some maximum value. The systems that remained stable during this stage became unstable to the anomalous Doppler or the Cerenkov resonances when the dc field was kept at the saturation level or decreased. Once the instability is triggered, the runaway tail is isotropized.

  6. Dynamics of runaway tails with time-dependent sub-Dreicer dc fields in magnetized plasmas

    SciTech Connect

    Moghaddam-Taaheri, E.; Vlahos, L.

    1987-10-01

    The evolution of runaway tails driven by sub-Dreicer time-dependent dc fields in a magnetized plasma are studied numerically using a quasilinear code based on the Ritz--Galerkin method and finite elements. It is found that the runaway tail maintained a negative slope during the dc field increase. Depending on the values of the dc electric field at t = 0 and the electron gyrofrequency to the plasma frequency ratio the runaway tail became unstable to the anomalous Doppler resonance or remained stable before the saturation of the dc field at some maximum value. The systems that remained stable during this stage became unstable to the anomalous Doppler or the C-hacekerenkov resonances when the dc field was kept at the saturation level or decreased. Once the instability is triggered, the runaway tail is isotropized.

  7. Three-dimensional, time-dependent simulation of a regenerative amplifier free-electron laser

    NASA Astrophysics Data System (ADS)

    Freund, H. P.; Nguyen, D. C.; Sprangle, P. A.; van der Slot, P. J. M.

    2013-01-01

    Free-electron lasers have been designed to operate over virtually the entire electromagnetic spectrum from microwaves through x rays and in a variety of configurations including amplifiers and oscillators. Oscillators typically operate in the low-gain regime where the full spectral width is (Δω/ω)≈1/Nw and the efficiency η≈1/(2.4Nw). Further, since a low-gain oscillator saturates when the gain compensates for losses in the resonator G=L/(1-L), this implies that the losses must be relatively small and the cavity Q must be relatively large. This imposes problems for high power oscillators because the high Q can result in mirror loading above the damage threshold, and in short-wavelength oscillators because sufficiently low loss resonators may not be possible at x-ray wavelengths. In contrast, regenerative amplifier FELs (RAFELs) employ high-gain wigglers that reach exponential gain and can operate with high loss (i.e., low Q) resonators. As such, RAFELs may be able to function at either high power levels or short wavelengths. In this paper, we describe a three-dimensional, time-dependent simulation of a RAFEL operating at a 2.2-μm wavelength, and show that its behavior differs substantially from that of low-gain oscillators, and is closer to that of self-amplified spontaneous radiation FELs in regard to spectral linewidth and extraction efficiency.

  8. Strong field ionization rates simulated with time-dependent configuration interaction and an absorbing potential

    SciTech Connect

    Krause, Pascal; Sonk, Jason A.; Schlegel, H. Bernhard

    2014-05-07

    Ionization rates of molecules have been modeled with time-dependent configuration interaction simulations using atom centered basis sets and a complex absorbing potential. The simulations agree with accurate grid-based calculations for the ionization of hydrogen atom as a function of field strength and for charge resonance enhanced ionization of H{sub 2}{sup +} as the bond is elongated. Unlike grid-based methods, the present approach can be applied to simulate electron dynamics and ionization in multi-electron polyatomic molecules. Calculations on HCl{sup +} and HCO{sup +} demonstrate that these systems also show charge resonance enhanced ionization as the bonds are stretched.

  9. A case of time-dependent anisotropy of low-field susceptibility (AMS)

    NASA Astrophysics Data System (ADS)

    Borradaile, Graham J.; Geneviciene, Ieva

    2007-07-01

    A suite of non-tectonized, Meso-Proterozoic siliceous crystal tuffs and volcanic breccia with a visible stratification has a modal bulk susceptibility ( k) ˜ 160 μSI [mean; S.D. = 141 μSI; 44 μSI]. Normally, such susceptibilities suffice to make reliable measurements of anisotropy of low field susceptibility (AMS) using AC induction-coil instruments. However, for this suite, time-dependent susceptibility - variations during measurement are large in comparison to susceptibility - differences along different axes through a specimen. Thus, in many specimens, AMS axes determined by routine induction coil measurement in a (Sapphire Instruments SI2B; 19,200 Hz, 60 A/m) measurement procedures are not reproducible. The apparent variation of specimen susceptibility during a single, four minute AMS measurement can > 2 μSI whereas in the same interval the noise-level of our instrument is < 0.2 μSI. Thus, the time-dependence of the specimen-susceptibility is an intrinsic phenomenon due to the characteristics (grain size, domain structure) of the magnetite which dominates susceptibility during measurement and handling. Two procedures improved the reproducibility and stability of AMS axial orientations in some specimens. First, for some specimens, one or two cycles of LTD or AF demagnetization (≤ 15 mT) stabilized AMS axes. (Previous workers have observed that LTD and AF demagnetization may change slightly the AMS of polydomainal magnetite). Of course, exposure to alternating fields is preferably avoided before any AMS study. Second, for some specimens AMS measurement were improved by shielding the induction coil instrument in a large magnetically shielded space (ambient field < 5 nT). Further improvements were achieved by permitting the specimens to relax in side a magnetic shield for 24 h before measurement. The occurrence of time-dependent bulk susceptibility, especially noticeable in its AMS axial orientations is certainly a rare phenomenon and the procedures we used

  10. Solvent effects in time-dependent self-consistent field methods. I. Optical response calculations

    DOE PAGES

    Bjorgaard, J. A.; Kuzmenko, V.; Velizhanin, K. A.; ...

    2015-01-22

    In this study, we implement and examine three excited state solvent models in time-dependent self-consistent field methods using a consistent formalism which unambiguously shows their relationship. These are the linear response, state specific, and vertical excitation solvent models. Their effects on energies calculated with the equivalent of COSMO/CIS/AM1 are given for a set of test molecules with varying excited state charge transfer character. The resulting solvent effects are explained qualitatively using a dipole approximation. It is shown that the fundamental differences between these solvent models are reflected by the character of the calculated excitations.

  11. Wave function for harmonically confined electrons in time-dependent electric and magnetostatic fields.

    PubMed

    Zhu, Hong-Ming; Chen, Jin-Wang; Pan, Xiao-Yin; Sahni, Viraht

    2014-01-14

    We derive via the interaction "representation" the many-body wave function for harmonically confined electrons in the presence of a magnetostatic field and perturbed by a spatially homogeneous time-dependent electric field-the Generalized Kohn Theorem (GKT) wave function. In the absence of the harmonic confinement - the uniform electron gas - the GKT wave function reduces to the Kohn Theorem wave function. Without the magnetostatic field, the GKT wave function is the Harmonic Potential Theorem wave function. We further prove the validity of the connection between the GKT wave function derived and the system in an accelerated frame of reference. Finally, we provide examples of the application of the GKT wave function.

  12. Linear-response time-dependent density-functional theory with pairing fields.

    PubMed

    Peng, Degao; van Aggelen, Helen; Yang, Yang; Yang, Weitao

    2014-05-14

    Recent development in particle-particle random phase approximation (pp-RPA) broadens the perspective on ground state correlation energies [H. van Aggelen, Y. Yang, and W. Yang, Phys. Rev. A 88, 030501 (2013), Y. Yang, H. van Aggelen, S. N. Steinmann, D. Peng, and W. Yang, J. Chem. Phys. 139, 174110 (2013); D. Peng, S. N. Steinmann, H. van Aggelen, and W. Yang, J. Chem. Phys. 139, 104112 (2013)] and N ± 2 excitation energies [Y. Yang, H. van Aggelen, and W. Yang, J. Chem. Phys. 139, 224105 (2013)]. So far Hartree-Fock and approximated density-functional orbitals have been utilized to evaluate the pp-RPA equation. In this paper, to further explore the fundamentals and the potential use of pairing matrix dependent functionals, we present the linear-response time-dependent density-functional theory with pairing fields with both adiabatic and frequency-dependent kernels. This theory is related to the density-functional theory and time-dependent density-functional theory for superconductors, but is applied to normal non-superconducting systems for our purpose. Due to the lack of the proof of the one-to-one mapping between the pairing matrix and the pairing field for time-dependent systems, the linear-response theory is established based on the representability assumption of the pairing matrix. The linear response theory justifies the use of approximated density-functionals in the pp-RPA equation. This work sets the fundamentals for future density-functional development to enhance the description of ground state correlation energies and N ± 2 excitation energies.

  13. Continuous surface switching: An improved time-dependent self-consistent-field method for nonadiabatic dynamics

    NASA Astrophysics Data System (ADS)

    Volobuev, Yuri L.; Hack, Michael D.; Topaler, Maria S.; Truhlar, Donald G.

    2000-06-01

    We present a new semiclassical method for electronically nonadiabatic collisions. The method is a variant of the time-dependent self-consistent-field method and is called continuous surface switching. The algorithm involves a self-consistent potential trajectory surface switching approach that is designed to combine the advantages of the trajectory surface hopping approach and the Ehrenfest classical path self-consistent potential approach without their relative disadvantages. Viewed from the self-consistent perspective, it corresponds to "on-the-fly histogramming" of the Ehrenfest method by a natural decay of mixing; viewed from the surface hopping perspective, it corresponds to replacing discontinuous surface hops by continuous surface switching. In this article we present the method and illustrate it for three multidimensional cases. Accurate quantum mechanical scattering calculations are carried out for these three cases by a linear algebraic variational method, and the accurate values of reactive probabilities, quenching probabilities, and moments of final vibrational and rotational distributions are compared to the results of continuous surface switching, the trajectory surface hopping method in two representations, the time-dependent self-consistent-field method, and the Miller-Meyer classical electron method to place the results of the semiclassical methods in perspective.

  14. Studies of time dependence of fields in TEVATRON superconducting dipole magnets

    SciTech Connect

    Hanft, R.W.; Brown, B.C.; Herrup, D.A.; Lamm, M.J.; McInturff, A.D.; Syphers, M.J.

    1988-08-22

    The time variation in the magnetic field of a model Tevatron dipole magnet at constant excitation current has been studied. Variations in symmetry allowed harmonic components over long time ranges show a log t behavior indicative of ''flux creep.'' Both short time range and long time range behavior depend in a detailed way on the excitation history. Similar effects are seen in the remnant fields present in full-scale Tevatron dipoles following current ramping. Both magnitudes and time dependences are observed to depend on details for the ramps, such as ramp rate, flattop duration, and number of ramps. In a few magnets, variations are also seen in symmetry unallowed harmonics. 9 refs., 10 figs.

  15. Mechanism of Electron Excitation and Emission from a Nanoribbon under Pulsed Laser Irradiation: Time-Dependent First-Principles Study

    NASA Astrophysics Data System (ADS)

    Miyauchi, Shota; Watanabe, Kazuyuki

    2017-03-01

    A time-dependent density functional theory simulation demonstrated the sequential dynamics of electron excitation and emission from a silicene nanoribbon under a femtosecond laser pulse. The mechanism for the multiphoton absorption processes that are responsible for the kinetic-energy spectra of emitted electrons was elucidated using Kohn-Sham potentials and the decomposition scheme.

  16. Interpreting quantum states of electromagnetic field in time-dependent linear media

    NASA Astrophysics Data System (ADS)

    Choi, Jeong Ryeol

    2010-11-01

    Recently, Pedrosa and Rosas [Phys. Rev. Lett.PRLTAO0031-900710.1103/PhysRevLett.103.010402 103, 010402 (2009)] investigated the quantum states of an electromagnetic field in time-dependent linear media using a Hermitian linear invariant. The wave function obtained by them is represented in terms of an arbitrary weight function g(λl). Since the type of wave function varies depending on the choice of g(λl) in their problem, it may be a difficult task to construct a coherent state that resembles the classical state from their theory. We suggest, on the basis of a non-Hermitian linear invariant, another quantum state that is a kind of coherent state. The expectation value of canonical variables in this alternate state follows an exact classical trajectory. For a simple case in which the time dependence of the parameters ɛ(t), μ(t), and σ(t) disappears, we showed that the quantum energy expectation value in the alternate quantum state recovers exactly to the classical energy in the limit ℏ→0. This alternate state leads to the correspondence between the quantum and the classical behaviors of physical observables in a high-energy limit.

  17. Driving self-assembly and emergent dynamics in colloidal suspensions by time-dependent magnetic fields

    DOE PAGES

    Martin, James E.; Snezhko, Alexey

    2013-11-05

    In this review we discuss recent research on driving self assembly of magnetic particle suspensions subjected to alternating magnetic fields. The variety of structures and effects that can be induced in such systems is remarkably broad due to the large number of variables involved. The alternating field can be uniaxial, biaxial or triaxial, the particles can be spherical or anisometric, and the suspension can be dispersed throughout a volume or confined to a soft interface. In the simplest case the field drives the static or quasi-static assembly of unusual particle structures, such as sheets, networks and open-cell foams. More complex,more » emergent collective behaviors evolve in systems that can follow the time-dependent field vector. In these cases energy is continuously injected into the system and striking °ow patterns and structures can arise. In fluid volumes these include the formation of advection and vortex lattices. At air-liquid and liquid-liquid interfaces striking dynamic particle assemblies emerge due to the particle-mediated coupling of the applied field to surface excitations. These out-of-equilibrium interface assemblies exhibit a number of remarkable phenomena, including self-propulsion and surface mixing. In addition to discussing various methods of driven self assembly in magnetic suspensions, some of the remarkable properties of these novel materials are described.« less

  18. Driving self-assembly and emergent dynamics in colloidal suspensions by time-dependent magnetic fields

    NASA Astrophysics Data System (ADS)

    Martin, James E.; Snezhko, Alexey

    2013-12-01

    In this review we discuss recent research on driving self-assembly of magnetic particle suspensions subjected to alternating magnetic fields. The variety of structures and effects that can be induced in such systems is remarkably broad due to the large number of variables involved. The alternating field can be uniaxial, biaxial or triaxial, the particles can be spherical or anisometric, and the suspension can be dispersed throughout a volume or confined to a soft interface. In the simplest case the field drives the static or quasistatic assembly of unusual particle structures, such as sheets, networks and open-cell foams. More complex, emergent collective behaviors evolve in systems that can follow the time-dependent field vector. In these cases energy is continuously injected into the system and striking flow patterns and structures can arise. In fluid volumes these include the formation of advection and vortex lattices. At air-liquid and liquid-liquid interfaces striking dynamic particle assemblies emerge due to the particle-mediated coupling of the applied field to surface excitations. These out-of-equilibrium interface assemblies exhibit a number of remarkable phenomena, including self-propulsion and surface mixing. In addition to discussing various methods of driven self-assembly in magnetic suspensions, some of the remarkable properties of these novel materials are described.

  19. Driving self-assembly and emergent dynamics in colloidal suspensions by time-dependent magnetic fields

    SciTech Connect

    Martin, James E.; Snezhko, Alexey

    2013-11-05

    In this review we discuss recent research on driving self assembly of magnetic particle suspensions subjected to alternating magnetic fields. The variety of structures and effects that can be induced in such systems is remarkably broad due to the large number of variables involved. The alternating field can be uniaxial, biaxial or triaxial, the particles can be spherical or anisometric, and the suspension can be dispersed throughout a volume or confined to a soft interface. In the simplest case the field drives the static or quasi-static assembly of unusual particle structures, such as sheets, networks and open-cell foams. More complex, emergent collective behaviors evolve in systems that can follow the time-dependent field vector. In these cases energy is continuously injected into the system and striking °ow patterns and structures can arise. In fluid volumes these include the formation of advection and vortex lattices. At air-liquid and liquid-liquid interfaces striking dynamic particle assemblies emerge due to the particle-mediated coupling of the applied field to surface excitations. These out-of-equilibrium interface assemblies exhibit a number of remarkable phenomena, including self-propulsion and surface mixing. In addition to discussing various methods of driven self assembly in magnetic suspensions, some of the remarkable properties of these novel materials are described.

  20. Modeling laser induced molecule excitation using real-time time-dependent density functional theory: application to 5- and 6-benzyluracil.

    PubMed

    Bende, Attila; Toşa, Valer

    2015-02-28

    The fully propagated real time-dependent density functional theory method has been applied to study the laser-molecule interaction in 5- and 6-benzyluracil (5BU and 6BU). The molecular geometry optimization and the time-dependent electronic dynamics propagation were carried out using the M11-L local meta-NGA (nonseparable gradient approximations) exchange-correlation functional together with the def2-TZVP basis set. Different laser field parameters like direction, strength, and wavelength have been varied in order to estimate the conditions for an efficient excitation of the molecules. The results show that the two molecules respond differently to the applied laser field and therefore specific laser field parameters have to be chosen for each of them in order to get efficient and selective excitation behavior. It was also found that from the molecular excitation point of view not only the magnitude of the transition dipoles between the involved orbitals but also their orientation with respect to the laser field is important. On the other hand, it was shown that the molecular excitation is a very complex overlapping of different one-electron orbital depopulation-population processes of the occupied and virtual orbitals.

  1. Dynamical Mean-Field Equations for a Neural Network with Spike Timing Dependent Plasticity

    NASA Astrophysics Data System (ADS)

    Mayer, Jörg; Ngo, Hong-Viet V.; Schuster, Heinz Georg

    2012-09-01

    We study the discrete dynamics of a fully connected network of threshold elements interacting via dynamically evolving synapses displaying spike timing dependent plasticity. Dynamical mean-field equations, which become exact in the thermodynamical limit, are derived to study the behavior of the system driven with uncorrelated and correlated Gaussian noise input. We use correlated noise to verify that our model gives account to the fact that correlated noise provides stronger drive for synaptic modification. Further we find that stochastic independent input leads to a noise dependent transition to the coherent state where all neurons fire together, most notably there exists an optimal noise level for the enhancement of synaptic potentiation in our model.

  2. Instabilities of thin layers of conducting fluids produced by time dependent magnetic fields

    NASA Astrophysics Data System (ADS)

    Burguete, Javier

    2011-11-01

    We present the recent results of an experiment where thin layers of conducting fluids are forced by time-dependent magnetic fields perpendicular to their surface. We use as conducting fluid an In-Ga-Sn alloy, immersed in a 5% hydrocloric acid solution to prevent oxidation. The conducting layers have a circular shape, and are placed inside a set-up that produces the vertical magnetic field. Due to MHD effects, the competition between the Lorentz force and gravity triggers an instability of the free surface. The shape of this surface can adopt many different configurations, with a very rich dynamics, presenting azimuthal wave numbers between 3 and 8 for the explored parameters. The magnetic field evolves harmonically with a frequency up to 10Hz, small enough to not to observe skin depth effects and with a magnitude up to 0.1 T. Different resonant regions have been observed, for narrow windows of the forcing frequency. We have analysed the existence of thresholds for these instabilities, depending on the wave number and experimental parameters. These results are compared with others present in the literature.

  3. Entanglement in a time-dependent coupled XY spin chain in an external magnetic field

    SciTech Connect

    Sadiek, Gehad; Alkurtass, Bedoor; Aldossary, Omar

    2010-11-15

    We consider an infinite one-dimensional anisotropic XY spin chain with a nearest-neighbor time-dependent Heisenberg coupling J(t) between the spins in presence of a time-dependent magnetic field h(t). We discuss a general solution for the system and present an exact solution for particular choice of J and h of practical interest. We investigate the dynamics of entanglement for different degrees of anisotropy of the system and at both zero and finite temperatures. We find that the time evolution of entanglement in the system shows nonergodic and critical behavior at zero and finite temperatures and different degrees of anisotropy. The asymptotic behavior of entanglement at the infinite time limit at zero temperature and constant J and h depends only the parameter {lambda}=J/h rather than the individual values of J and h for all degrees of anisotropy but changes for nonzero temperature. Furthermore, the asymptotic behavior is very sensitive to the initial values of J and h and for particular choices we may create finite asymptotic entanglement regardless of the final values of J and h. The persistence of quantum effects in the system as it evolves and as the temperature is raised is studied by monitoring the entanglement. We find that the quantum effects dominate within certain regions of the kT-{lambda} space that vary significantly depending on the degree of the anisotropy of the system. Particularly, the quantum effects in the Ising model case persist in the vicinity of both its critical phase transition point and zero temperature as it evolves in time. Moreover, the interplay between the different system parameters to tune and control the entanglement evolution is explored.

  4. Light cone in the two-dimensional transverse-field Ising model in time-dependent mean-field theory

    NASA Astrophysics Data System (ADS)

    Hafner, J.; Blass, B.; Rieger, H.

    2016-12-01

    We investigate the propagation of a local perturbation in the two-dimensional transverse-field Ising model with a time-dependent application of the mean-field theory based on the BBGKY hierarchy. We show that the perturbation propagates through the system with a finite velocity and that there is a transition from Manhattan to Euclidian metric, resulting in a light cone with an almost circular shape at sufficiently large distances. The propagation velocity of the perturbation defining the front of the light cone is discussed with respect to the parameters of the Hamiltonian and compared to exact results for the transverse-field Ising model in one dimension.

  5. Time-dependent flow fields around the spherical colonial alga Volvox carteri

    NASA Astrophysics Data System (ADS)

    Brumley, Douglas; Polin, Marco; Morez, Constant; Goldstein, Raymond; Pedley, Timothy

    2011-11-01

    Volvox carteri is a spherical colonial alga, consisting of thousands of biflagellate cells. The somatic cells embedded on the surface of the colony beat their flagella approximately towards the south pole, producing a net fluid motion. Using high-speed imaging and particle image velocimetry (PIV) we have been able to accurately analyse the time-dependent flow fields around such colonies. The somatic cells on the colony surface may beat their flagella in a perfectly synchronised fashion, or may exhibit behaviour in which the coordination wanders periodically between forward and backward propagating metachronal waves. We analyse the dependence of this synchronisation on fundamental parameters in the system such as colony radius, characterise the speed and wavelength of metachronal waves propagating on the surface, and investigate the extent to which hydrodynamic interactions are responsible for the exhibited behaviour. The time-averaged flow fields agree with previous experiments involving freely swimming colonies (Phys. Rev. Lett. 105:168101, 2010) and Blake's squirmer model (J. Fluid Mech. 46, 199-208, 1971b).

  6. Time-dependent density functional theory of high-intensity short-pulse laser irradiation on insulators

    NASA Astrophysics Data System (ADS)

    Sato, S. A.; Yabana, K.; Shinohara, Y.; Otobe, T.; Lee, K.-M.; Bertsch, G. F.

    2015-11-01

    We calculate the energy deposition by very short laser pulses in SiO2 (α -quartz) with a view to establishing systematics for predicting damage and nanoparticle production. The theoretical framework is time-dependent density functional theory, implemented by the real-time method in a multiscale representation. For the most realistic simulations we employ a meta-GGA Kohn-Sham potential similar to that of Becke and Johnson. We find that the deposited energy in the medium can be accurately modeled as a function of the local electromagnetic pulse fluence. The energy-deposition function can in turn be quite well fitted to the strong-field Keldysh formula for a range of intensities from below the melting threshold to well beyond the ablation threshold. We find reasonable agreement between the damage threshold and the energy required to melt the substrate. Also, the depth of the ablated crater at higher energies is fairly well reproduced assuming that the material ablated with the energy exceeds that required to convert it to an atomic fluid. However, the calculated ablation threshold is higher than experiment, suggesting a nonthermal mechanism for the surface ablation.

  7. Three-dimensional, time-dependent simulation of free-electron lasers with planar, helical, and elliptical undulators

    NASA Astrophysics Data System (ADS)

    Freund, H. P.; van der Slot, P. J. M.; Grimminck, D. L. A. G.; Setija, I. D.; Falgari, P.

    2017-02-01

    Free-electron lasers (FELs) have been built ranging in wavelength from long-wavelength oscillators using partial wave guiding through ultraviolet through hard x-ray that are either seeded or start from noise. In addition, FELs that produce different polarizations of the output radiation ranging from linear through elliptic to circular polarization are currently under study. In this paper, we develop a three-dimensional, time-dependent formulation that is capable of modeling this large variety of FEL configurations including different polarizations. We employ a modal expansion for the optical field, i.e., a Gaussian expansion with variable polarization for free-space propagation. This formulation uses the full Newton–Lorentz force equations to track the particles through the optical and magnetostatic fields. As a result, arbitrary three-dimensional representations for different undulator configurations are implemented, including planar, helical, and elliptical undulators. In particular, we present an analytic model of an APPLE-II undulator to treat arbitrary elliptical polarizations, which is used to treat general elliptical polarizations. To model oscillator configurations, and allow propagation of the optical field outside the undulator and interact with optical elements, we link the FEL simulation with the optical propagation code OPC. We present simulations using the APPLE-II undulator model to produce elliptically polarized output radiation, and present a detailed comparison with recent experiments using a tapered undulator configuration at the Linac Coherent Light Source. Validation of the nonlinear formation is also shown by comparison with experimental results obtained in the Sorgente Pulsata Auto-amplificata di Radiazione Coerente SASE FEL experiment at ENEA Frascati, a seeded tapered amplifier experiment at Brookhaven National Laboratory, and the 10 kW upgrade oscillator experiment at the Thomas Jefferson National Accelerator Facility.

  8. A pseudospectral matrix method for time-dependent tensor fields on a spherical shell

    SciTech Connect

    Brügmann, Bernd

    2013-02-15

    We construct a pseudospectral method for the solution of time-dependent, non-linear partial differential equations on a three-dimensional spherical shell. The problem we address is the treatment of tensor fields on the sphere. As a test case we consider the evolution of a single black hole in numerical general relativity. A natural strategy would be the expansion in tensor spherical harmonics in spherical coordinates. Instead, we consider the simpler and potentially more efficient possibility of a double Fourier expansion on the sphere for tensors in Cartesian coordinates. As usual for the double Fourier method, we employ a filter to address time-step limitations and certain stability issues. We find that a tensor filter based on spin-weighted spherical harmonics is successful, while two simplified, non-spin-weighted filters do not lead to stable evolutions. The derivatives and the filter are implemented by matrix multiplication for efficiency. A key technical point is the construction of a matrix multiplication method for the spin-weighted spherical harmonic filter. As example for the efficient parallelization of the double Fourier, spin-weighted filter method we discuss an implementation on a GPU, which achieves a speed-up of up to a factor of 20 compared to a single core CPU implementation.

  9. Microscopic theory of dissipation for slowly time-dependent mean field potentials

    NASA Astrophysics Data System (ADS)

    Aleshin, V. P.

    2005-10-01

    We study the dissipation rate Q˙ in systems of nucleons bound by a slowly time-dependent mean-field potential and slightly interacting between themselves. Starting from the many-body linear response formula we evaluate an expression for Q˙ in terms of the pure shell-model quantities and the nucleon-nucleon collision rate Γ. The application of the classical sum rule leads then to an expression for Q˙ in terms of the classical-path integral with the weighting function including Γ. For vanishing Γ this expression reduces to the Koonin-Randrup Knudsen-gas formula. For simplified Skyrme interactions the classical approximation for the Γ itself is obtained. In leptodermous systems the classical-path expression for Q˙ decomposes into the wall formula and the multiple-reflection term owing to incomplete randomization of particle motion between consecutive encounters with the boundary. The mean-free path and temperature dependence of dissipation is analyzed for small-amplitude distortions of spherical cavities.

  10. Time-dependent restricted-active-space self-consistent-field theory with space partition

    NASA Astrophysics Data System (ADS)

    Miyagi, Haruhide; Madsen, Lars Bojer

    2017-02-01

    Aiming at efficient numerical analysis of time-dependent (TD) many-electron dynamics of atoms involving multielectron continua, the TD restricted-active-space self-consistent-field theory with space partition (TD-RASSCF-SP) is presented. The TD-RASSCF-SP wave function is expanded in terms of TD configuration-interaction coefficients with Slater determinants composed of two kinds of TD orbitals: M ̂ orbitals are defined to be nonvanishing in the inner region (V ̂), a small volume around the atomic nucleus, and M ˇ orbitals are nonvanishing in the large outer region (V ˇ). For detailed discussion of the SP strategy, the equations of motion are derived by two different formalisms for comparison. To ensure continuous differentiability of the wave function across the two regions, one of the formalisms makes use of the property of the finite-element discrete-variable-representation (FEDVR) functions and introduces additional time-independent orbitals. The other formalism is more general and is based on the Bloch operator as in the R -matrix theory, but turns out to be less practical for numerical applications. Hence, using the FEDVR-based formalism, the numerical performance is tested by computing double-ionization dynamics of atomic beryllium in intense light fields. To achieve high accuracy, M ̂ should be set large to take into account the strong many-electron correlation around the nucleus. On the other hand, M ˇ can be set much smaller than M ̂ for capturing the weaker correlation between the two outgoing photoelectrons. As a result, compared with more accurate multiconfigurational TD Hartree-Fock (MCTDHF) method, the TD-RASSCF-SP method may achieve comparable accuracy in the description of the double-ionization dynamics. There are, however, difficulties related to the stiffness of the equations of motion of the TD-RASSCF-SP method, which makes the required time step for this method smaller than the one needed for the MCTDHF approach.

  11. Time-dependent energetic proton acceleration and scaling laws in ultraintense laser-pulse interactions with thin foils.

    PubMed

    Huang, Yongsheng; Bi, Yuanjie; Shi, Yijin; Wang, Naiyan; Tang, Xiuzhang; Gao, Zhe

    2009-03-01

    A two-phase model, where the plasma expansion is an isothermal one when laser irradiates and a following adiabatic one after laser ends, has been proposed to predict the maximum energy of the proton beams induced in the ultraintense laser-foil interactions. The hot-electron recirculation in the ultraintense laser-solid interactions has been accounted in and described by the time-dependent hot-electron density continuously in this model. The dilution effect of electron density as electrons recirculate and spread laterally has been considered. With our model, the scaling laws of maximum ion energy have been achieved and the dependence of the scaling coefficients on laser intensity, pulse duration, and target thickness have been obtained. Some interesting results have been predicted: the adiabatic expansion is an important process of the ion acceleration and cannot be neglected; the whole acceleration time is about 10-20 times of laser-pulse duration; the larger the laser intensity, the more sensitive the maximum ion energy to the change of focus radius, and so on.

  12. Time-Dependent, Three-Dimensional Simulation of Free-Electron-Laser Oscillators

    SciTech Connect

    Slot, P. J. M. van der; Boller, K.-J.; Freund, H. P.; Miner, W. H. Jr.; Benson, S. V.; Shinn, M.

    2009-06-19

    We describe a procedure for the simulation of free-electron-laser (FEL) oscillators. The simulation uses a combination of the MEDUSA simulation code for the FEL interaction and the OPC code to model the resonator. The simulations are compared with recent observations of the oscillator at the Thomas Jefferson National Accelerator Facility and are in substantial agreement with the experiment.

  13. Time-dependent dynamics of intense laser-induced above threshold Coulomb explosion

    NASA Astrophysics Data System (ADS)

    Esry, B. D.; Ben-Itzhak, I.

    2007-06-01

    We use our recently proposed model [1] to extract information about the nuclear dynamics from the recent Coulomb explosion data of Staudte et al. taken with 40 fs pulses [2]. That data, taken at multiple intensities near the ionization appearance intensity for both H2 and D2 in linearly and circularly polarized light, shows remarkable structure and regularity not easily explained by conventional models. Because our model does fit the spectra well, we can infer the qualitative time-dependent evolution of the system. In addition, we speculate about the possibility of rescattering leading to above threshold Coulomb explosion. [1] B.D. Esry, A.M. Sayler, P.Q. Wang, K.D. Carnes, and I. Ben-Itzhak, Phys. Rev. Lett. 97, 013003 (2006). [2] A. Staudte, D. Pavici'c, S. Chelkowski, D. Zeidler, M. Meckel, H. Niikura, M. Sch"offler, S. Sch"ossler, B. Ulrich, P. P. Rajeev, Th. Weber, T. Jahnke, D.M. Villeneuve, A.D. Bandrauk, C.L. Cocke, P.B. Corkum, and R. D"orner, Phys. Rev. Lett. (accepted).

  14. Laser-induced electron dynamics including photoionization: A heuristic model within time-dependent configuration interaction theory.

    PubMed

    Klinkusch, Stefan; Saalfrank, Peter; Klamroth, Tillmann

    2009-09-21

    We report simulations of laser-pulse driven many-electron dynamics by means of a simple, heuristic extension of the time-dependent configuration interaction singles (TD-CIS) approach. The extension allows for the treatment of ionizing states as nonstationary states with a finite, energy-dependent lifetime to account for above-threshold ionization losses in laser-driven many-electron dynamics. The extended TD-CIS method is applied to the following specific examples: (i) state-to-state transitions in the LiCN molecule which correspond to intramolecular charge transfer, (ii) creation of electronic wave packets in LiCN including wave packet analysis by pump-probe spectroscopy, and, finally, (iii) the effect of ionization on the dynamic polarizability of H(2) when calculated nonperturbatively by TD-CIS.

  15. Time-Dependent Propagation of High-Energy Laser Beams Through the Atmosphere: III

    DTIC Science & Technology

    2007-11-02

    Hermann . 7 This method assumes the phase correction to be proportional to the thermally- induced density change at the transmitter. The constant of...field amplitude & is assumed to satisfy the Helmholtz equation in Fresnel approximation 2ik^ = vH +k28e& , (10) oz 1 14 where the intensity

  16. Quantum work statistics of charged Dirac particles in time-dependent fields

    DOE PAGES

    Deffner, Sebastian; Saxena, Avadh

    2015-09-28

    The quantum Jarzynski equality is an important theorem of modern quantum thermodynamics. We show that the Jarzynski equality readily generalizes to relativistic quantum mechanics described by the Dirac equation. After establishing the conceptual framework we solve a pedagogical, yet experimentally relevant, system analytically. As a main result we obtain the exact quantum work distributions for charged particles traveling through a time-dependent vector potential evolving under Schrödinger as well as under Dirac dynamics, and for which the Jarzynski equality is verified. Thus, special emphasis is put on the conceptual and technical subtleties arising from relativistic quantum mechanics.

  17. Quantum work statistics of charged Dirac particles in time-dependent fields

    NASA Astrophysics Data System (ADS)

    Deffner, Sebastian; Saxena, Avadh

    2015-09-01

    The quantum Jarzynski equality is an important theorem of modern quantum thermodynamics. We show that the Jarzynski equality readily generalizes to relativistic quantum mechanics described by the Dirac equation. After establishing the conceptual framework we solve a pedagogical, yet experimentally relevant, system analytically. As a main result we obtain the exact quantum work distributions for charged particles traveling through a time-dependent vector potential evolving under Schrödinger as well as under Dirac dynamics, and for which the Jarzynski equality is verified. Special emphasis is put on the conceptual and technical subtleties arising from relativistic quantum mechanics.

  18. Effect of the time-dependent coupling on a superconducting qubit-field system under decoherence: Entanglement and Wehrl entropy

    SciTech Connect

    Abdel-Khalek, S.; Berrada, K.; Eleuch, H.

    2015-10-15

    The dynamics of a superconducting (SC) qubit interacting with a field under decoherence with and without time-dependent coupling effect is analyzed. Quantum features like the collapse–revivals for the dynamics of population inversion, sudden birth and sudden death of entanglement, and statistical properties are investigated under the phase damping effect. Analytic results for certain parametric conditions are obtained. We analyze the influence of decoherence on the negativity and Wehrl entropy for different values of the physical parameters. We also explore an interesting relation between the SC-field entanglement and Wehrl entropy behavior during the time evolution. We show that the amount of SC-field entanglement can be enhanced as the field tends to be more classical. The studied model of SC-field system with the time-dependent coupling has high practical importance due to their experimental accessibility which may open new perspectives in different tasks of quantum formation processing.

  19. Systematic study of low-lying E1 strength using the time-dependent mean field theory

    SciTech Connect

    Ebata, S.; Nakatsukasa, T.; Inakura, T.

    2012-11-12

    We carry out systematic investigation of electric dipole (E1) mode from light to heavy nuclei, using a new time-dependent mean field theory: the Canonical-basis Time-Dependent Hartree-Fock-Bogoliubov (Cb-TDHFB) theory. The Cb-TDHFB in the three-dimensional coordinate space representation can deal with pairing correlation and any kind of deformation in the timedependent framework. We report the neutron-number dependence of the low-energy E1 mode for light (A > 40) and heavy isotopes (A < 100) around N= 82.

  20. Quantum work statistics of charged Dirac particles in time-dependent fields

    NASA Astrophysics Data System (ADS)

    Deffner, Sebastian; Saxena, Avadh

    The quantum Jarzynski equality is an important theorem of modern quantum thermodynamics. We show that the Jarzynski equality readily generalizes to relativistic quantum mechanics described by the Dirac equation. After establishing the conceptual framework we solve a pedagogical, yet experimentally relevant, system analytically. As a main result we obtain the exact quantum work distributions for charged particles traveling through a time-dependent vector potential evolving under Schrödinger as well as under Dirac dynamics, and for which the Jarzynski equality is verified. Special emphasis is put on the conceptual and technical subtleties arising from relativistic quantum mechanics. SD acknowledges financial support by the U.S. Department of Energy through a LANL Director's Funded Fellowship.

  1. Analytical solutions for anisotropic time-dependent heat equations with Robin boundary condition for cubic-shaped solid-state laser crystals.

    PubMed

    Sabaeian, Mohammad

    2012-10-20

    The problem of finding analytical solutions for time-dependent or time-independent heat equations, especially for solid-state laser media, has required a lot of work in the field of thermal effects. However, to calculate the temperature distributions analytically, researchers often have to make some approximations or employ complex methods. In this work, we present full analytical solutions for anisotropic time-dependent heat equations in the Cartesian coordinates with various source terms corresponding to various pumping schemes. Moreover, the most general boundary condition of Robin (or impedance boundary condition), corresponding to the convection cooling mechanism, was applied. This general condition can be easily switched to constant temperature and thermal insulation as special cases. To this end, we first proposed a general approach to solving time-dependent heat equations with an arbitrary heat source. We then applied our approach to explore the temperature distribution for three cases: steady-state pumping or long transient, single-shot pumping or short transient, and repetitively pulsed pumping. Our results show the possibility of an easier and more accurate approach to analytical calculations of the thermal dispersion, thermal stresses (strains), thermal bending, thermal phase shift, and other thermal effects.

  2. Near-field: a finite-difference time-dependent method for simulation of electrodynamics on small scales.

    PubMed

    Coomar, Arunima; Arntsen, Christopher; Lopata, Kenneth A; Pistinner, Shlomi; Neuhauser, Daniel

    2011-08-28

    We develop near-field (NF), a very efficient finite-difference time-dependent (FDTD) approach for simulating electromagnetic systems in the near-field regime. NF is essentially a time-dependent version of the quasistatic frequency-dependent Poisson algorithm. We assume that the electric field is longitudinal, and hence propagates only a set of time-dependent polarizations and currents. For near-field scales, the time step (dt) is much larger than in the usual Maxwell FDTD approach, as it is not related to the velocity of light; rather, it is determined by the rate of damping and plasma oscillations in the material, so dt = 2.5 a.u. was well converged in our simulations. The propagation in time is done via a leapfrog algorithm much like Yee's method, and only a single spatial convolution is needed per time step. In conjunction, we also develop a new and very accurate 8 and 9 Drude-oscillators fit to the permittivity of gold and silver, desired here because we use a large time step. We show that NF agrees with Mie-theory in the limit of small spheres and that it also accurately describes the evolution of the spectral shape as a function of the separation between two gold or silver spheres. The NF algorithm is especially efficient for systems with small scale dynamics and makes it very simple to introduce additional effects such as embedding.

  3. On the integration of fields and quanta in time dependent backgrounds

    NASA Astrophysics Data System (ADS)

    Castillo, Esteban; Koch, Benjamin; Palma, Gonzalo

    2014-05-01

    Field theories with global continuous symmetries may admit configurations in which time translation invariance is broken by the movement of homogeneous background fields evolving along the flat directions implied by the symmetries. In this context, the field fluctuations along the broken symmetry are well parametrized by a Goldstone boson field that may non-trivially interact with other fields present in the theory. These interactions violate Lorentz invariance as a result of the broken time translation invariance of the background, producing a mixing between the field content and the particle spectrum of the theory. In this article we study the effects of such interactions on the low energy dynamics of the Goldstone boson quanta, paying special attention to the role of the particle spectrum of the theory. By studying the particular case of a canonical two-field model with a mexican-hat potential, we analyze the derivation of the low energy effective field theory for the Goldstone boson, and discuss in detail the distinction between integrating fields v/s integrating quanta, to finally conclude that they are equivalent. In addition, we discuss the implications of our analysis for the study of systems where time translation invariance is broken, such as cosmic inflation and time crystals.

  4. Time-dependent behavior of magnetic fields confined by conducting walls

    SciTech Connect

    Kidder, R.E.; Cecil, A.B.

    1983-03-09

    An equation is derived which describes the total current flowing in a moving conducting surface surrounding a magnetic field, where diffusion of the field into the conductor is taken into account. Analytic and numerical solutions of the current equation are obtained for the cases of exponential and linear compression of the magnetic field with time, respectively. It is assumed that the electrical conductivity is constant, that the conducting surfaces are axially symmetric, and that the thickness and radius of curvature of the conducting walls is large compared with the effective depth of penetration of the field.

  5. Barriers to transport in aperiodically time-dependent two-dimensional velocity fields: Nekhoroshev's theorem and "Nearly Invariant" tori

    NASA Astrophysics Data System (ADS)

    Wiggins, S.; Mancho, A. M.

    2014-02-01

    In this paper we consider fluid transport in two-dimensional flows from the dynamical systems point of view, with the focus on elliptic behaviour and aperiodic and finite time dependence. We give an overview of previous work on general nonautonomous and finite time vector fields with the purpose of bringing to the attention of those working on fluid transport from the dynamical systems point of view a body of work that is extremely relevant, but appears not to be so well known. We then focus on the Kolmogorov-Arnold-Moser (KAM) theorem and the Nekhoroshev theorem. While there is no finite time or aperiodically time-dependent version of the KAM theorem, the Nekhoroshev theorem, by its very nature, is a finite time result, but for a "very long" (i.e. exponentially long with respect to the size of the perturbation) time interval and provides a rigorous quantification of "nearly invariant tori" over this very long timescale. We discuss an aperiodically time-dependent version of the Nekhoroshev theorem due to Giorgilli and Zehnder (1992) (recently refined by Bounemoura, 2013 and Fortunati and Wiggins, 2013) which is directly relevant to fluid transport problems. We give a detailed discussion of issues associated with the applicability of the KAM and Nekhoroshev theorems in specific flows. Finally, we consider a specific example of an aperiodically time-dependent flow where we show that the results of the Nekhoroshev theorem hold.

  6. Destabilizing effect of time-dependent oblique magnetic field on magnetic fluids streaming in porous media.

    PubMed

    El-Dib, Yusry O; Ghaly, Ahmed Y

    2004-01-01

    The present work studies Kelvin-Helmholtz waves propagating between two magnetic fluids. The system is composed of two semi-infinite magnetic fluids streaming throughout porous media. The system is influenced by an oblique magnetic field. The solution of the linearized equations of motion under the boundary conditions leads to deriving the Mathieu equation governing the interfacial displacement and having complex coefficients. The stability criteria are discussed theoretically and numerically, from which stability diagrams are obtained. Regions of stability and instability are identified for the magnetic fields versus the wavenumber. It is found that the increase of the fluid density ratio, the fluid velocity ratio, the upper viscosity, and the lower porous permeability play a stabilizing role in the stability behavior in the presence of an oscillating vertical magnetic field or in the presence of an oscillating tangential magnetic field. The increase of the fluid viscosity plays a stabilizing role and can be used to retard the destabilizing influence for the vertical magnetic field. Dual roles are observed for the fluid velocity in the stability criteria. It is found that the field frequency plays against the constant part for the magnetic field.

  7. Time-dependent Suppression of Oscillatory Power in Evolving Solar Magnetic Fields

    NASA Astrophysics Data System (ADS)

    Krishna Prasad, S.; Jess, D. B.; Jain, R.; Keys, P. H.

    2016-05-01

    Oscillation amplitudes are generally smaller within magnetically active regions like sunspots and plage when compared to their surroundings. Such magnetic features, when viewed in spatially resolved power maps, appear as regions of suppressed power due to reductions in the oscillation amplitudes. Employing high spatial- and temporal-resolution observations from the Dunn Solar Telescope (DST) in New Mexico, we study the power suppression in a region of evolving magnetic fields adjacent to a pore. By utilizing wavelet analysis, we study for the first time how the oscillatory properties in this region change as the magnetic field evolves with time. Image sequences taken in the blue continuum, G-band, Ca ii K, and Hα filters were used in this study. It is observed that the suppression found in the chromosphere occupies a relatively larger area, confirming previous findings. Also, the suppression is extended to structures directly connected to the magnetic region, and is found to get enhanced as the magnetic field strength increased with time. The dependence of the suppression on the magnetic field strength is greater at longer periods and higher formation heights. Furthermore, the dominant periodicity in the chromosphere was found to be anti-correlated with increases in the magnetic field strength.

  8. Time-dependent perturbation of a two-state quantum system by a sinusoidal field

    NASA Technical Reports Server (NTRS)

    Dion, D. R.; Hirschfelder, J. O.

    1976-01-01

    Different methods for solving the 'two-level problem' are discussed, namely, the problem of what happens to a material system having only two nondegenerate energy levels when it is perturbed by an electromagnetic field that varies with time in a monochromatic sinusoidal fashion. The various methods discussed include: (1) the Sen Gupta technique using nondegenerate Rayleigh-Schroedinger perturbation theory, (2) the Salwen-Winter-Shirley partitioning perturbation technique, (3) the Shirley and series degenerate Rayleigh-Schroedinger expansion, (4) the degenerate Rayleigh-Schroedinger technique for considering high frequency fields, and (5) the singular perturbation expansion technique.

  9. Quantum logic gates from time-dependent global magnetic field in a system with constant exchange

    SciTech Connect

    Nenashev, A. V. Dvurechenskii, A. V.; Zinovieva, A. F.; Gornov, A. Yu.; Zarodnyuk, T. S.

    2015-03-21

    We propose a method that implements a universal set of one- and two-quantum-bit gates for quantum computation in a system of coupled electron pairs with constant non-diagonal exchange interaction. In our proposal, suppression of the exchange interaction is performed by the continual repetition of single-spin rotations. A small g-factor difference between the electrons allows for addressing qubits and avoiding strong magnetic field pulses. Numerical experiments were performed to show that, to implement the one- and two-qubit operations, it is sufficient to change the strength of the magnetic field by a few Gauss. This introduces one and then the other electron in a resonance. To determine the evolution of the two-qubit system, we use the algorithms of optimal control theory.

  10. Time dependence of 50 Hz magnetic fields in apartment buildings with indoor transformer stations.

    PubMed

    Yitzhak, Nir-Mordechay; Hareuveny, Ronen; Kandel, Shaiela; Ruppin, Raphael

    2012-04-01

    Twenty-four hour measurements of 50 Hz magnetic fields (MFs) in apartment buildings containing transformer stations have been performed. The apartments were classified into four types, according to their location relative to the transformer room. Temporal correlation coefficients between the MF in various apartments, as well as between MF and transformer load curves, were calculated. It was found that, in addition to their high average MF, the apartments located right above the transformer room also exhibit unique temporal correlation properties.

  11. Pseudo-Steady Diffusional Growth or Collapse of Bubbles Rising in Time Dependent Pressure Fields

    DTIC Science & Technology

    1990-03-13

    et al. [12], Ishikawa, et al. [13] and Payvar [14] to name a few. Brankovic, et al. collected data for air and carbon dioxide bubbles with a triple...hydrostatic pressure field. Payvar [141 examined the effects, both experimentally and analytically, of a rapid de- compression on bubble growth for C0 2...Furthermore, bubble experimental rise data have only been obtained for a static hydrostatic head, with the exception of Payvar [14], but that was for a

  12. A time-dependent Ginzburg-Landau phase field formalism for shock-induced phase transitions

    NASA Astrophysics Data System (ADS)

    Haxhimali, Tomorr; Belof, Jonathan L.; Benedict, Lorin X.

    2017-01-01

    Phase-field models have become popular in the last two decades to describe a host of free-boundary problems. The strength of the method relies on implicitly describing the dynamics of surfaces and interfaces by a continuous scalar field that enters the global grand free energy functional of the system. Here we explore the potential utility of this method in order to describe shock-induced phase transitions. To this end we make use of the Multiphase Field Theory (MFT) to account for the existence of multiple phases during the transition, and we couple MFT to a hydrodynamic model in the context of a new LLNL code for phase transitions, SAMSA. As a demonstration of this approach, we apply our code to the α - ɛ-Fe phase transition under shock wave loading conditions and compare our results with experiments of Jensen et. al. [J. Appl. Phys., 105:103502 (2009)] and Barker and Hollenbach [J. Appl. Phys., 45:4872 (1974)].

  13. Time-dependent low-field MRI characteristics of canine blood: an in vitro study.

    PubMed

    Jeong, Jimo; Park, Sangjun; Jeong, Eunseok; Kim, Namsoo; Kim, Minsu; Jung, Yechan; Cho, Youngkwon; Lee, Kichang

    2016-03-01

    This study was conducted to assess time-sensitive magnetic resonance (MR) changes in canine blood using low-field MR. Arterial and venous blood samples were collected from eight healthy beagle dogs. Samples were placed in 5-mL tubes and imaged within 3 hours of collection at 1 day intervals from day 1 to day 30. The following sequences were used: T1-weighted (T1W), T2-weighted (T2W), fluid-attenuated inversion recovery (FLAIR), short tau inversion recovery (STIR), and T2-star gradient-echo (T2(*)-GRE). Visual comparison of the images revealed that four relatively homogenous blood clots and twelve heterogeneous blood clots developed. The margination of the clot and plasma changed significantly on day 2 and day 13. On day 2, heterogeneous blood clots were differentiated into 2 to 3 signal layers in the T2W, T1W, and especially the STIR images. Hypointense signal layers were also detected in the blood clots in STIR images, which have T2 hypo, FLAIR hypo, and T1 hyper intense signals. In all images, these signal layers remained relatively unchanged until day 13. Overall, the results suggest that hematomas are complex on low-field MRI. Accordingly, it may not be feasible to accurately characterize hemorrhages and predict clot age based on low-field MRI.

  14. Anomalous transport in fluid field with random waiting time depending on the preceding jump length

    NASA Astrophysics Data System (ADS)

    Zhang, Hong; Li, Guo-Hua

    2016-11-01

    Anomalous (or non-Fickian) transport behaviors of particles have been widely observed in complex porous media. To capture the energy-dependent characteristics of non-Fickian transport of a particle in flow fields, in the present paper a generalized continuous time random walk model whose waiting time probability distribution depends on the preceding jump length is introduced, and the corresponding master equation in Fourier-Laplace space for the distribution of particles is derived. As examples, two generalized advection-dispersion equations for Gaussian distribution and lévy flight with the probability density function of waiting time being quadratic dependent on the preceding jump length are obtained by applying the derived master equation. Project supported by the Foundation for Young Key Teachers of Chengdu University of Technology, China (Grant No. KYGG201414) and the Opening Foundation of Geomathematics Key Laboratory of Sichuan Province, China (Grant No. scsxdz2013009).

  15. Time-dependent complete-active-space self-consistent-field method for atoms: Application to high-order harmonic generation

    NASA Astrophysics Data System (ADS)

    Sato, Takeshi; Ishikawa, Kenichi L.; Březinová, Iva; Lackner, Fabian; Nagele, Stefan; Burgdörfer, Joachim

    2016-08-01

    We present a numerical implementation of the time-dependent complete-active-space self-consistent-field (TD-CASSCF) method [Phys. Rev. A 88, 023402 (2013), 10.1103/PhysRevA.88.023402] for atoms driven by a strong linearly polarized laser pulse. The present implementation treats the problem in its full dimensionality and introduces a gauge-invariant frozen-core approximation, an efficient evaluation of the Coulomb mean field scaling linearly with the number of basis functions, and a split-operator method specifically designed for stable propagation of stiff spatial derivative operators. We apply this method to high-harmonic generation in helium, beryllium, and neon and explore the role of electron correlations.

  16. Paramagnetic Meissner effect and strong time dependence at high fields in melt-textured high- T C superconductors

    NASA Astrophysics Data System (ADS)

    de Paiva Gouvêa, Cristol; Dias, Fábio Teixeira; das Neves Vieira, Valdemar; da Silva, Douglas Langie; Schaf, Jacob; Wolff-Fabris, Frederik; Rovira, Joan Josep Roa

    2013-05-01

    In this work we report on systematic field-cooled magnetization experiments in melt-textured YBa2Cu3O7- δ samples containing Y211 precipitates. Magnetic fields up to 14 T were applied either parallel or perpendicular to the ab planes and a strong paramagnetic response related to the superconducting state was observed. This effect is known as paramagnetic Meissner effect (PME). The magnitude of the PME increases when the field is augmented. This effect shows a strong paramagnetic relaxation, such that the paramagnetic moment increases as a function of the time. The pinning by the Y211 particles plays a crucial role in the explanation of this effect and our results suggest that the pinning capacity can produce a strong flux compression into the sample, originating the PME and the strong time dependence.

  17. Time dependent wind fields

    NASA Technical Reports Server (NTRS)

    Chelton, D. B.

    1986-01-01

    Two tasks were performed: (1) determination of the accuracy of Seasat scatterometer, altimeter, and scanning multichannel microwave radiometer measurements of wind speed; and (2) application of Seasat altimeter measurements of sea level to study the spatial and temporal variability of geostrophic flow in the Antarctic Circumpolar Current. The results of the first task have identified systematic errors in wind speeds estimated by all three satellite sensors. However, in all cases the errors are correctable and corrected wind speeds agree between the three sensors to better than 1 ms sup -1 in 96-day 2 deg. latitude by 6 deg. longitude averages. The second task has resulted in development of a new technique for using altimeter sea level measurements to study the temporal variability of large scale sea level variations. Application of the technique to the Antarctic Circumpolar Current yielded new information about the ocean circulation in this region of the ocean that is poorly sampled by conventional ship-based measurements.

  18. Solvent effects in time-dependent self-consistent field methods. II. Variational formulations and analytical gradients

    SciTech Connect

    Bjorgaard, J. A.; Velizhanin, K. A.; Tretiak, S.

    2015-08-06

    This study describes variational energy expressions and analytical excited state energy gradients for time-dependent self-consistent field methods with polarizable solvent effects. Linear response, vertical excitation, and state-specific solventmodels are examined. Enforcing a variational ground stateenergy expression in the state-specific model is found to reduce it to the vertical excitation model. Variational excited state energy expressions are then provided for the linear response and vertical excitation models and analytical gradients are formulated. Using semiempiricalmodel chemistry, the variational expressions are verified by numerical and analytical differentiation with respect to a static external electric field. Lastly, analytical gradients are further tested by performing microcanonical excited state molecular dynamics with p-nitroaniline.

  19. Solvent effects in time-dependent self-consistent field methods. II. Variational formulations and analytical gradients

    DOE PAGES

    Bjorgaard, J. A.; Velizhanin, K. A.; Tretiak, S.

    2015-08-06

    This study describes variational energy expressions and analytical excited state energy gradients for time-dependent self-consistent field methods with polarizable solvent effects. Linear response, vertical excitation, and state-specific solventmodels are examined. Enforcing a variational ground stateenergy expression in the state-specific model is found to reduce it to the vertical excitation model. Variational excited state energy expressions are then provided for the linear response and vertical excitation models and analytical gradients are formulated. Using semiempiricalmodel chemistry, the variational expressions are verified by numerical and analytical differentiation with respect to a static external electric field. Lastly, analytical gradients are further tested by performingmore » microcanonical excited state molecular dynamics with p-nitroaniline.« less

  20. Theoretical Shaping of Femtosecond Laser Pulses for Molecular Photodissociation with Control Techniques Based on Ehrenfest's Dynamics and Time-Dependent Density Functional Theory.

    PubMed

    Castro, Alberto

    2016-06-03

    The combination of nonadiabatic Ehrenfest-path molecular dynamics (EMD) based on time-dependent density functional theory (TDDFT) and quantum optimal control formalism (QOCT) was used to optimize the shape of ultra-short laser pulses to achieve photodissociation of a hydrogen molecule and the trihydrogen cation H3 (+) . This work completes a previous one [A. Castro, ChemPhysChem, 2013, 14, 1488-1495], in which the same objective was achieved by demonstrating the combination of QOCT and TDDFT for many-electron systems on static nuclear potentials. The optimization model, therefore, did not include the nuclear movement and the obtained dissociation mechanism could only be sequential: fast laser-assisted electronic excitation to nonbonding states (during which the nuclei are considered to be static), followed by field-free dissociation. Here, in contrast, the optimization was performed with the QOCT constructed on top of the full dynamic model comprised of both electrons and nuclei, as described within EMD based on TDDFT. This is the first numerical demonstration of an optimal control formalism for a hybrid quantum-classical model, that is, a molecular dynamics method.

  1. Time-dependent configuration-interaction calculations of laser-pulse-driven many-electron dynamics: Controlled dipole switching in lithium cyanide

    NASA Astrophysics Data System (ADS)

    Krause, Pascal; Klamroth, Tillmann; Saalfrank, Peter

    2005-08-01

    We report simulations of laser-driven many-electron dynamics by means of the time-dependent configuration interaction singles (doubles) approach. The method accounts for the correlation of ground and excited states, is capable of describing explicitly time-dependent, nonlinear phenomena, and is systematically improvable. Lithium cyanide serves as a molecular test system in which the charge distribution and hence the dipole moment are shown to be switchable, in a controlled fashion, by (a series of) laser pulses which induce selective, state-to-state electronic transitions. One focus of our time-dependent calculations is the question of how fast the transition from the ionic ground state to a specific excited state that is embedded in a multitude of other states can be made, without creating an electronic wave packet.

  2. Excitation dynamics in a lattice Bose gas within the time-dependent Gutzwiller mean-field approach

    SciTech Connect

    Krutitsky, Konstantin V.; Navez, Patrick

    2011-09-15

    The dynamics of the collective excitations of a lattice Bose gas at zero temperature is systematically investigated using the time-dependent Gutzwiller mean-field approach. The excitation modes are determined within the framework of the linear-response theory as solutions of the generalized Bogoliubov-de Gennes equations valid in the superfluid and Mott-insulator phases at arbitrary values of parameters. The expression for the sound velocity derived in this approach coincides with the hydrodynamic relation. We calculate the transition amplitudes for the excitations in the Bragg scattering process and show that the higher excitation modes make significant contributions. We simulate the dynamics of the density perturbations and show that their propagation velocity in the limit of week perturbation is satisfactorily described by the predictions of the linear-response analysis.

  3. Strong-field ionization rates of linear polyenes simulated with time-dependent configuration interaction with an absorbing potential.

    PubMed

    Krause, Pascal; Schlegel, H Bernhard

    2014-11-07

    The strong field ionization rates for ethylene, trans 1,3-butadiene, and trans,trans 1,3,5-hexatriene have been calculated using time-dependent configuration interaction with single excitations and a complex absorbing potential (TDCIS-CAP). The calculations used the aug-cc-pVTZ basis set with a large set of diffuse functions (3 s, 2 p, 3 d, and 1 f) on each atom. The absorbing boundary was placed 3.5 times the van der Waals radius from each atom. The simulations employed a seven-cycle cosine squared pulse with a wavelength of 800 nm. Ionization rates were calculated for intensities ranging from 0.3 × 10(14) W/cm(2) to 3.5 × 10(14) W/cm(2). Ionization rates along the molecular axis increased markedly with increasing conjugation length. By contrast, ionization rates perpendicular to the molecular axis were almost independent of the conjugation length.

  4. Strong-field ionization rates of linear polyenes simulated with time-dependent configuration interaction with an absorbing potential

    NASA Astrophysics Data System (ADS)

    Krause, Pascal; Schlegel, H. Bernhard

    2014-11-01

    The strong field ionization rates for ethylene, trans 1,3-butadiene, and trans,trans 1,3,5-hexatriene have been calculated using time-dependent configuration interaction with single excitations and a complex absorbing potential (TDCIS-CAP). The calculations used the aug-cc-pVTZ basis set with a large set of diffuse functions (3 s, 2 p, 3 d, and 1 f) on each atom. The absorbing boundary was placed 3.5 times the van der Waals radius from each atom. The simulations employed a seven-cycle cosine squared pulse with a wavelength of 800 nm. Ionization rates were calculated for intensities ranging from 0.3 × 1014 W/cm2 to 3.5 × 1014 W/cm2. Ionization rates along the molecular axis increased markedly with increasing conjugation length. By contrast, ionization rates perpendicular to the molecular axis were almost independent of the conjugation length.

  5. Dynamical quantum-electrodynamics embedding: combining time-dependent density functional theory and the near-field method.

    PubMed

    Gao, Yi; Neuhauser, Daniel

    2012-08-21

    We develop an approach for dynamical (ω > 0) embedding of mixed quantum mechanical (QM)/classical (or more precisely QM/electrodynamics) systems with a quantum sub-region, described by time-dependent density functional theory (TDDFT), within a classical sub-region, modeled here by the recently proposed near-field (NF) method. Both sub-systems are propagated simultaneously and are coupled through a common Coulomb potential. As a first step we implement the method to study the plasmonic response of a metal film which is half jellium-like QM and half classical. The resulting response is in good agreement with both full-scale TDDFT and the purely classical NF method. The embedding method is able to describe the optical response of the whole system while capturing quantum mechanical effects, so it is a promising approach for studying electrodynamics in hybrid molecules-metals nanostructures.

  6. Linear scaling solution of the time-dependent self-consistent-field equations with quasi-independent Rayleigh quotient iteration

    SciTech Connect

    Challacombe, Matt

    2009-01-01

    An algorithm for solution of the Time-Dependent Self-Consistent-Field (TD-SCF) equations is developed, based on dual solution channels for non-linear optimization of the Tsiper functional [J.Phys.B, 34 L401 (2001)]. This formulation poses the TD-SCF problem as two Rayleigh quotients, coupled weakly through biorthogonality. Convergence rates for the Random Phase Approximation (RPA) are found to be equivalent to the Tamm-Dancoff approximation (TDA). Moreover, the variational nature of the quotient is robust to approximation errors, allowing linear scaling solution to the bulk limit of the RPA matrix-eigenvalue and exchange operator problem for molecular wires with extended conjugation, including polyphenylene vinylene and the (4,3) nanotube.

  7. Quantum/classical time-dependent self-consistent field treatment of Ar+HCO inelastic and dissociative scattering

    NASA Astrophysics Data System (ADS)

    Whittier, Gregory S.; Light, John C.

    1999-03-01

    A quantum/classical time-dependent self-consistent field (Q/C TDSCF) approach is used to simulate the dynamics of collisions of Ar with HCO. We present state-to-state cross sections and thermal rate constants for vibrational transitions. Using this model together with assumptions about the rotational energy transfer and a master equation treatment of the kinetics, the low-pressure thermal rate of collision-induced dissociation (CID) was calculated over the 300-4000 K temperature range. A comparison with experiment shows good agreement at high temperatures and poor agreement at low temperatures. The high temperature results were sufficient to obtain an Arrhenius expression for the rate that agrees with all experimental results of which we are aware.

  8. Time-dependent analytical R-matrix approach for strong-field dynamics. I. One-electron systems

    NASA Astrophysics Data System (ADS)

    Torlina, Lisa; Smirnova, Olga

    2012-10-01

    We develop a flexible analytical approach to describe strong-field dynamics in atoms and molecules. The approach is based on the ideas of the R-matrix method. Here, we illustrate and validate our approach by applying it to systems with one active electron bound by the Coulomb potential and benchmark our results against the standard theory of Perelomov, Popov, and Terent'ev [Sov. Phys. JETP0021-903710.1007/BF01132710 23, 924 (1966)]. We discuss corrections to the ionization amplitude associated with the interplay of the Coulomb potential and the laser field on the sub-laser cycle time scale and the shape of the tunneling wave packets associated with different instants of ionization.

  9. Time-dependent scattering theory for charged Dirac fields on a Reissner-Nordström black hole

    NASA Astrophysics Data System (ADS)

    Thierry, Daudé

    2010-10-01

    In this paper, we prove a complete time-dependent scattering theory for charged (massive or not) Dirac fields outside a Reissner-Nordström black hole. We shall take the point of view of observers static at infinity, well described by the Schwarzschild system of coordinates. For such observers, the exterior of a Reissner-Nordström black hole is a smooth manifold having two distinct asymptotic regions: the horizon and spacelike infinity. We first simplify the later analysis using the spherical symmetry of the Reissner-Nordström black hole and we reduce the initial 3+1 dimensional evolution equation of hyperbolic type into a 1+1 dimensional one. Then, we establish various propagation estimates for such fields in the same spirit as in the works by Dereziński and Gérard [Scattering Theory of Classical and Quantum N-Particle Systems (Springer-Verlag, Berlin, 1997)]. We construct the asymptotic velocity operators P+/- and we show that their spectra are equal to σ(P+)={-1}∪[0,1] and σ(P-)=[-1,0]∪{1}. This information points out the very distinct behaviors of Dirac fields near the two asymptotic regions of the black hole. As a consequence of this construction, we prove the existence and asymptotic completeness of (Dollard modified at infinity) wave operators.

  10. SVD-Based Technique for Interference Cancellation and Noise Reduction in NMR Measurement of Time-Dependent Magnetic Fields

    PubMed Central

    Chen, Wenjun; Ma, Hong; Yu, De; Zhang, Hua

    2016-01-01

    A nuclear magnetic resonance (NMR) experiment for measurement of time-dependent magnetic fields was introduced. To improve the signal-to-interference-plus-noise ratio (SINR) of NMR data, a new method for interference cancellation and noise reduction (ICNR) based on singular value decomposition (SVD) was proposed. The singular values corresponding to the radio frequency interference (RFI) signal were identified in terms of the correlation between the FID data and the reference data, and then the RFI and noise were suppressed by setting the corresponding singular values to zero. The validity of the algorithm was verified by processing the measured NMR data. The results indicated that, this method has a significantly suppression of RFI and random noise, and can well preserve the FID signal. At present, the major limitation of the proposed SVD-based ICNR technique is that the threshold value for interference cancellation needs to be manually selected. Finally, the inversion waveform of the applied alternating magnetic field was given by fitting the processed experimental data. PMID:26959024

  11. SVD-Based Technique for Interference Cancellation and Noise Reduction in NMR Measurement of Time-Dependent Magnetic Fields.

    PubMed

    Chen, Wenjun; Ma, Hong; Yu, De; Zhang, Hua

    2016-03-04

    A nuclear magnetic resonance (NMR) experiment for measurement of time-dependent magnetic fields was introduced. To improve the signal-to-interference-plus-noise ratio (SINR) of NMR data, a new method for interference cancellation and noise reduction (ICNR) based on singular value decomposition (SVD) was proposed. The singular values corresponding to the radio frequency interference (RFI) signal were identified in terms of the correlation between the FID data and the reference data, and then the RFI and noise were suppressed by setting the corresponding singular values to zero. The validity of the algorithm was verified by processing the measured NMR data. The results indicated that, this method has a significantly suppression of RFI and random noise, and can well preserve the FID signal. At present, the major limitation of the proposed SVD-based ICNR technique is that the threshold value for interference cancellation needs to be manually selected. Finally, the inversion waveform of the applied alternating magnetic field was given by fitting the processed experimental data.

  12. Time-dependent Induced Seismicity Rates Described with an Epidemic Type Aftershock Sequence Model at The Geysers Geothermal Field, California

    NASA Astrophysics Data System (ADS)

    Johnson, C. W.; Totten, E. J.; Burgmann, R.

    2015-12-01

    To improve understanding of the link between injection/production activity and seismicity, we apply an Epidemic Type Aftershock Sequence (ETAS) model to an earthquake catalog from The Geysers geothermal field (GGF) between 2005-2015 using >140,000 events and Mc 0.8 . We partition the catalog along a northeast-southwest trending divide, which corresponds to regions of high and low levels of enhanced geothermal stimulation (EGS) across the field. The ETAS model is fit to the seismicity data using a 6-month sliding window with a 1-month time step to determine the background seismicity rate. We generate monthly time series of the time-dependent background seismicity rate in 1-km depth intervals from 0-5km. The average wellhead depth is 2-3 km and the background seismicity rates above this depth do not correlate well with field-wide injected masses over the time period of interest. The auto correlation results show a 12-month period for monthly time series proximal to the average wellhead depths (2-3km and 3-4km) for northwest GGF strongly correlates with field-wide fluid injection masses, with a four-month phase shift between the two depth intervals as fluid migrates deeper. This periodicity is not observed for the deeper depth interval of 4-5 km, where monthly background seismicity rates reduce to near zero. Cross-correlation analysis using the monthly time series for background seismicity rate and the field-wide injection, production and net injection (injection minus production) suggest that injection most directly modulates seismicity. Periodicity in the background seismicity is not observed as strongly in the time series for the southeast field. We suggest that the variation in background seismicity rate is a proxy for pore-pressure diffusion of injected fluids at depth. We deduce that the contrast between the background seismicity rates in the northwest and southeast GGF is a result of reduced EGS activity in the southeast region.

  13. First principles calculation of field emission from nanostructures using time-dependent density functional theory: A simplified approach

    NASA Astrophysics Data System (ADS)

    Tawfik, Sherif A.; El-Sheikh, S. M.; Salem, N. M.

    2011-05-01

    We introduce a new simplified method for computing the electron field emission current in short carbon nanotubes and graphene sheets using ab-initio computation in slab-periodic simulation cells. The evolution of the wave functions using Time-Dependent Density Functional Theory is computed by utilizing the Crank-Nicholson propagator and using the Octopus code (Castro et al., 2006 [1]), where we skip the wave function relaxation step elaborated by Han et al. (2002) [2], and apply a norm-conserving wave propagation method instead of the norm-nonconserving seventh-order Taylor Expansion method used by Araidai et al. (2004) [3]. Our method is mainly geared towards reducing the time it takes to compute the wave function propagation and enhancing the calculation precision. We found that in pristine carbon nanotubes, the emitted charge tends to emerge mostly from electrons that are concentrated at the nanotube tip region. The charge beam concentrates into specific channel structures, showing the utility of carbon nanotubes in precision emission applications.

  14. Strong-field ionization rates of linear polyenes simulated with time-dependent configuration interaction with an absorbing potential

    SciTech Connect

    Krause, Pascal; Schlegel, H. Bernhard

    2014-11-07

    The strong field ionization rates for ethylene, trans 1,3-butadiene, and trans,trans 1,3,5-hexatriene have been calculated using time-dependent configuration interaction with single excitations and a complex absorbing potential (TDCIS-CAP). The calculations used the aug-cc-pVTZ basis set with a large set of diffuse functions (3 s, 2 p, 3 d, and 1 f) on each atom. The absorbing boundary was placed 3.5 times the van der Waals radius from each atom. The simulations employed a seven-cycle cosine squared pulse with a wavelength of 800 nm. Ionization rates were calculated for intensities ranging from 0.3 × 10{sup 14} W/cm{sup 2} to 3.5 × 10{sup 14} W/cm{sup 2}. Ionization rates along the molecular axis increased markedly with increasing conjugation length. By contrast, ionization rates perpendicular to the molecular axis were almost independent of the conjugation length.

  15. Time dependence of the field energy densities surrounding sources: Application to scalar mesons near point sources and to electromagnetic fields near molecules

    NASA Astrophysics Data System (ADS)

    Persico, F.; Power, E. A.

    1987-07-01

    The time dependence of the dressing-undressing process, i.e., the acquiring or losing by a source of a boson field intensity and hence of a field energy density in its neighborhood, is considered by examining some simple soluble models. First, the loss of the virtual field is followed in time when a point source is suddenly decoupled from a neutral scalar meson field. Second, an initially bare point source acquires a virtual meson cloud as the coupling is switched on. The third example is that of an initially bare molecule interacting with the vacuum of the electromagnetic field to acquire a virtual photon cloud. In all three cases the dressing-undressing is shown to take place within an expanding sphere of radius r=ct centered at the source. At each point in space the energy density tends, for large times, to that of the ground state of the total system. Differences in the time dependence of the dressing between the massive scalar field and the massless electromagnetic field are discussed. The results are also briefly discussed in the light of Feinberg's ideas on the nature of half-dressed states in quantum field theory.

  16. Color opponent receptive fields self-organize in a biophysical model of visual cortex via spike-timing dependent plasticity

    PubMed Central

    Eguchi, Akihiro; Neymotin, Samuel A.; Stringer, Simon M.

    2014-01-01

    Although many computational models have been proposed to explain orientation maps in primary visual cortex (V1), it is not yet known how similar clusters of color-selective neurons in macaque V1/V2 are connected and develop. In this work, we address the problem of understanding the cortical processing of color information with a possible mechanism of the development of the patchy distribution of color selectivity via computational modeling. Each color input is decomposed into a red, green, and blue representation and transmitted to the visual cortex via a simulated optic nerve in a luminance channel and red–green and blue–yellow opponent color channels. Our model of the early visual system consists of multiple topographically-arranged layers of excitatory and inhibitory neurons, with sparse intra-layer connectivity and feed-forward connectivity between layers. Layers are arranged based on anatomy of early visual pathways, and include a retina, lateral geniculate nucleus, and layered neocortex. Each neuron in the V1 output layer makes synaptic connections to neighboring neurons and receives the three types of signals in the different channels from the corresponding photoreceptor position. Synaptic weights are randomized and learned using spike-timing-dependent plasticity (STDP). After training with natural images, the neurons display heightened sensitivity to specific colors. Information-theoretic analysis reveals mutual information between particular stimuli and responses, and that the information reaches a maximum with fewer neurons in the higher layers, indicating that estimations of the input colors can be done using the output of fewer cells in the later stages of cortical processing. In addition, cells with similar color receptive fields form clusters. Analysis of spiking activity reveals increased firing synchrony between neurons when particular color inputs are presented or removed (ON-cell/OFF-cell). PMID:24659956

  17. Estimation of a Time-Dependent Strain Rate Field in Southern California Using Continuous GPS Stations in the SCIGN Network.

    NASA Astrophysics Data System (ADS)

    Hernandez, D.; Holt, W. E.; Bennett, R. A.; Li, C.; Dimitrova, L. L.; Haines, A. J.

    2005-12-01

    Advancements in the recognition of fine-scale deformation fluctuations have prompted a great deal of attention to be focused on identifying and characterizing transient strain phenomena. We have developed a tool for recognizing strain rate transients as well as for quantifying the magnitude and style of their temporal and spatial variations. Using time-varying velocity estimates for continuous GPS station data from the Southern California Integrated GPS Network (SCIGN) for the time period between October 1999 and February 2004 [Li et al., 2005]. We determine time-averaged velocity values in 0.05 year epochs for each continuous velocity series. For each velocity field solution we determine a self-consistent model velocity gradient tensor field solution for the region using bi-cubic Bessel interpolation of the GPS velocity vectors. For each epoch solution we plot dilatation strain rates, shear strain rates, and the rotation rates. We also investigate the departures of the model strain rate field and velocity field from a master solution, obtained from a time-averaged solution for the period 1999-2004, as well as estimating the departures of the time variable velocity gradient tensor field from other master solutions, including models that incorporate plate motion constraints and Quaternary fault data. By combining the epoch solution plots, we create movies that allow us to view the spatial and temporal changes in the dilation and shear strain rate field in southern California. In the present solution several time-dependent changes are noteworthy. The Eastern California Shear Zone (ECSZ) region, immediately following the October 1999 Hector Mine earthquake, shows a significant spatial change of relatively high shear strain rate that increases from the immediate area of the earthquake to an area that almost spans the entire ECSZ from east to west. Also following the Hector Mine event, there is a strain rate corridor that extends through the Pinto Mt. fault connecting

  18. Time dependent holography

    NASA Astrophysics Data System (ADS)

    Das, Diptarka

    One of the most important results emerging from string theory is the gauge gravity duality (AdS/CFT correspondence) which tells us that certain problems in particular gravitational backgrounds can be exactly mapped to a particular dual gauge theory a quantum theory very similar to the one explaining the interactions between fundamental subatomic particles. The chief merit of the duality is that a difficult problem in one theory can be mapped to a simpler and solvable problem in the other theory. The duality can be used both ways. Most of the current theoretical framework is suited to study equilibrium systems, or systems where time dependence is at most adiabatic. However in the real world, systems are almost always out of equilibrium. Generically these scenarios are described by quenches, where a parameter of the theory is made time dependent. In this dissertation I describe some of the work done in the context of studying quantum quench using the AdS/CFT correspondence. We recover certain universal scaling type of behavior as the quenching is done through a quantum critical point. Another question that has been explored in the dissertation is time dependence of the gravity theory. Present cosmological observations indicate that our universe is accelerating and is described by a spacetime called de-Sitter(dS). In 2011 there had been a speculation over a possible duality between de-Sitter gravity and a particular field theory (Euclidean SP(N) CFT). However a concrete realization of this proposition was still lacking. Here we explicitly derive the dS/CFT duality using well known methods in field theory. We discovered that the time dimension emerges naturally in the derivation. We also describe further applications and extensions of dS/CFT. KEYWORDS: Holography, AdS/CFT correspondence, Quantum Quench, dS/CFT correspondence, Chaos.

  19. Methodology for determining time-dependent mechanical properties of tuff subjected to near-field repository conditions

    SciTech Connect

    Blacic, J.D.; Andersen, R.

    1983-01-01

    We have established a methodology to determine the time dependence of strength and transport properties of tuff under conditions appropriate to a nuclear waste repository. Exploratory tests to determine the approximate magnitudes of thermomechanical property changes are nearly complete. In this report we describe the capabilities of an apparatus designed to precisely measure the time-dependent deformation and permeability of tuff at simulated repository conditions. Preliminary tests with this new apparatus indicate that microclastic creep failure of tuff occurs over a narrow strain range with little precursory Tertiary creep behavior. In one test, deformation under conditions of slowly decreasing effective pressure resulted in failure, whereas some strain indicators showed a decreasing rate of strain.

  20. Time-dependent drift Hamiltonian

    SciTech Connect

    Boozer, A.H.

    1983-03-01

    The lowest-order drift equations are given in a canonical magnetic coordinate form for time-dependent magnetic and electric fields. The advantages of the canonical Hamiltonian form are also discussed.

  1. Time dependent diffraction ring patterns in bromothymol blue dye doped PMMA film under irradiation with continuous wave green laser light

    NASA Astrophysics Data System (ADS)

    Al-Saymari, F. A.; Badran, H. A.; Al-Ahmad, A. Y.; Emshary, C. A.

    2013-11-01

    Diffraction ring patterns are generated in bromothymol blue (BTB) doped poly methyl methacrylate (PMMA) film with the aid of visible light from a solid state laser of Gaussian distribution. Temporal evolution of patterns i.e. the number of rings increases as time elapse is observed. Based on the experimental findings, change in refractive index ( ∆n) effective nonlinear refractive index ( n 2) and variation of refractive index with temperature ( dn/ dT) have been obtained as 0.0025, 1.45 × 10-6 cm2 W-1, 1.69 × 10-5 K-1 respectively. Obtained results suggest the possibility of using BTB doped PMMA in data storage, recording and holography.

  2. Time dependent view factor methods

    SciTech Connect

    Kirkpatrick, R.C.

    1998-03-01

    View factors have been used for treating radiation transport between opaque surfaces bounding a transparent medium for several decades. However, in recent years they have been applied to problems involving intense bursts of radiation in enclosed volumes such as in the laser fusion hohlraums. In these problems, several aspects require treatment of time dependence.

  3. The weak field approximation and the strong field approximation for a quantum mechanical two-state system with an applied time-dependent force

    NASA Astrophysics Data System (ADS)

    Ropiak, Cynthia Ann

    A semi-classical treatment of the two-state atom subjected to a time-dependent applied force leads to a set of two coupled, complex, first-order ordinary differential equations governing the time evolution of the system's state vector that are to date, not solvable in closed form. Contained in this paper is a demonstration of how the system is parameterized by a single variable Θ, which in turn reduces the problem to one real, nonlinear, second-order ordinary differential equation. Utilizing a non-standard perturbation expansion in the variable `A' (the Field Strength Parameter) on this reduction subsequently allows for both a first-order Weak Field Approximation and a first-order Strong Field Approximation. In addition, a technique is outlined for obtaining the full power series solution in the Weak Field Limit (|A|<< l). However, a detailed discussion of the power series solution as well as its consequences is deferred due to the fact that it is presently a collaborative work in progress between Dr. Robert L. Anderson and myself. When applied to the specific case of both resonant and near-resonant linearly polarized light incident on an atom, both the Weak Field Approximation and the Strong Field Approximation are shown to be in good agreement with numerically generated solutions for the probability amplitudes of the state vector. Furthermore, this new Weak Field Approximation reveals the defect in the ansatz of discarding the `rapidly oscillating' term in the traditional Rotating Wave Approximation. Finally, the resonance case of the first-order Weak Field Approximation is found to contain large-time behavior. This large-time behavior is extracted and the new approximation is referred to as the Long-Time Weak Field Approximation. The resonance power series solution is demonstrated to contain large-time behavior, which is found to reduce to the first-order Long-Time Weak Field Approximation, but again a detailed analysis of the power series is deferred.

  4. Time-dependent oxidation during nano-assisted laser desorption ionization mass spectrometry: a useful tool for structure determination or a source of possible confusion?

    PubMed

    Pavlásková, Katerina; Strnadová, Marcela; Strohalm, Martin; Havlícek, Vladimír; Sulc, Miroslav; Volný, Michael

    2011-07-15

    This work reports on a new and extremely simple approach for determination of a double bond position by a laser desorption ionization mass spectrometry. It is solely based on the catalytic properties of nanostructured surfaces used in nanoassisted laser desorption ionization experiments. These surfaces can induce oxidation of analytes, which results in a mass shift that can be detected by mass spectrometry. If a site of unsaturation is oxidized and cleaved, the m/z difference is diagnostic of the position of a double bond. By demonstrating that the oxidation depends on the analyte surface dwell time, it was proven that it is caused by the surface activity and not by the laser desorption ionization process itself. Control matrix-assisted laser desorption/ionization (MALDI) experiment showed only a limited partial oxidation and no time dependency of the process. The ability to determine a position of a double bond was demonstrated on polyunsaturated phospholipids and cyclosporine A. In some other cases, however, the unexpected oxidation could cause confusion, as demonstrated for a glycosphingolipid from a porcine brain extract.

  5. Controlling the high frequency response of H{sub 2} by ultra-short tailored laser pulses: A time-dependent configuration interaction study

    SciTech Connect

    Schönborn, Jan Boyke; Saalfrank, Peter; Klamroth, Tillmann

    2016-01-28

    We combine the stochastic pulse optimization (SPO) scheme with the time-dependent configuration interaction singles method in order to control the high frequency response of a simple molecular model system to a tailored femtosecond laser pulse. For this purpose, we use H{sub 2} treated in the fixed nuclei approximation. The SPO scheme, as similar genetic algorithms, is especially suited to control highly non-linear processes, which we consider here in the context of high harmonic generation. Here, we will demonstrate that SPO can be used to realize a “non-harmonic” response of H{sub 2} to a laser pulse. Specifically, we will show how adding low intensity side frequencies to the dominant carrier frequency of the laser pulse and stochastically optimizing their contribution can create a high-frequency spectral signal of significant intensity, not harmonic to the carrier frequency. At the same time, it is possible to suppress the harmonic signals in the same spectral region, although the carrier frequency is kept dominant during the optimization.

  6. Status Report on the Modeling of TRISO Energy Deposition, Time-Dependent Temperature Field and Doppler Feedback

    SciTech Connect

    Javier Ortensi; Abderrafi M Ougouag

    2009-07-01

    The Doppler feedback mechanism is a major contributor to the passive safety of gas-cooled, graphite-moderated high temperature reactors that use fuel based on Tristructural-Isotropic coated particles. It follows that the correct prediction of the magnitude and time-dependence of this feedback effect is essential to the conduct of safety analyses for these reactors. We present a fuel conduction model for obtaining better estimates of the temperature feedback during moderate and fast transients. The fuel model has been incorporated in the CYNOD-THERMIX-KONVEK suite of coupled codes as a single TRISO particle within each calculation cell. The heat generation rate is scaled down from the neutronic solution and a Dirichlet boundary condition is imposed as the bulk graphite temperature from the thermal-hydraulic solution. This simplified approach yields similar results to those obtained with more complex methods, requiring multi-TRISO calculations within one control volume, but with much less computational effort. We provide an analysis of the hypothetical total control ejection event in the PBMR-400 design that clearly depicts the improvement in the predictions of the fuel temperature.

  7. Theoretical shaping of femtosecond laser pulses for ultrafast molecular photo-dissociation with control techniques based on time-dependent density functional theory.

    PubMed

    Castro, Alberto

    2013-05-10

    The combination of time-dependent density functional theory and quantum optimal control formalism is used to optimize the shape of ultra-short laser pulses in order to achieve the photodissociation of the hydrogen molecule. The very short pulse durations used in this work (a few femtoseconds) do not allow for significant nuclear movement during irradiation, and thus the dissociation mechanism is sequential. During pulse irradiation, a large sudden momentum is communicated which can be understood in terms of population of excited, bound or unbound, dissociative electronic states. The target is defined in terms of the average opposing force during the action of the pulse, or equivalently, in terms of the final dissociative velocity.

  8. Studies of Cosmic Ray Modulation and Energetic Particle Propagation in Time-Dependent 3-Dimensional Heliospheric Magnetic Fields

    NASA Technical Reports Server (NTRS)

    Zhang, Ming

    2005-01-01

    The primary goal of this project was to perform theoretical calculations of propagation of cosmic rays and energetic particles in 3-dimensional heliospheric magnetic fields. We used Markov stochastic process simulation to achieve to this goal. We developed computation software that can be used to study particle propagation in, as two examples of heliospheric magnetic fields that have to be treated in 3 dimensions, a heliospheric magnetic field suggested by Fisk (1996) and a global heliosphere including the region beyond the termination shock. The results from our model calculations were compared with particle measurements from Ulysses, Earth-based spacecraft such as IMP-8, WIND and ACE, Voyagers and Pioneers in outer heliosphere for tests of the magnetic field models. We particularly looked for features of particle variations that can allow us to significantly distinguish the Fisk magnetic field from the conventional Parker spiral field. The computer code will eventually lead to a new generation of integrated software for solving complicated problems of particle acceleration, propagation and modulation in realistic 3-dimensional heliosphere of realistic magnetic fields and the solar wind with a single computation approach.

  9. Time-dependent Ginzburg-Landau type Multiphase Field for description of shock-induced Phase Transition

    NASA Astrophysics Data System (ADS)

    Haxhimali, Tomorr; Belof, Jonathan; Benedict, Lorin

    2015-06-01

    Phase-field models have become popular in last two decades to describe a host of free-boundary problems. The strength of the method relies on implicitly describing the dynamics of surfaces and interfaces by continuous scalar field that enter in the global grand free energy functional of the system. We adapt this method in order to describe shock-induced phase transition. To this end we make use of the Multiphase Field Theory (MFT) to account for the existence of multiple phases during the transition. In this talk I will initially describe the constitutive equations that couple the dynamic of the phase field with that of the thermodynamic fields like T, P, c etc. I will then give details on developing a thermodynamically consistent phase-field interpolation function for multiple-phase system in the context of shock-induced phase-transition. At the end I will briefly comment on relating the dynamics of the interfaces in the shock/ramp compression to the Kardar-Parisi-Zhang equation. This work is performed under the auspices of the U. S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  10. Time-dependent modeling of field-aligned current-generated ion transients in the polar wind

    NASA Technical Reports Server (NTRS)

    Gombosi, T. I.; Nagy, A. F.

    1989-01-01

    The time evolution of field-aligned current-generated transient features in the high-latitude ionosphere is investigated. Ionospheric return currents generate significant downward heavy ion flows in the topside ionosphere with peak values well exceeding 10 to the 8th sq cm/s. When the return current ceases, the polar ionosphere rapidly returns to its previous equilibrium state. During the recovery phase of the return current event, an upward propagating heavy ion transient is formed, which is mainly characterized by a relatively short O(+) upwelling event. On the other hand, the H(+) escape flux remains relatively constant (within 10-20 percent) during field-aligned current events. It is also found that upward currents generate a transient heavy ion outflow, which exceeds the ambient H(+) escape flux by a factor of 3 to 5, depending on the duration and strength of the field-aligned current event.

  11. First-order quantum correction to the Larmor radiation from a moving charge in a spatially homogeneous time-dependent electric field

    SciTech Connect

    Yamamoto, Kazuhiro; Nakamura, Gen

    2011-02-15

    First-order quantum correction to the Larmor radiation is investigated on the basis of the scalar QED on a homogeneous background of a time-dependent electric field, which is a generalization of a recent work by Higuchi and Walker so as to be extended for an accelerated charged particle in a relativistic motion. We obtain a simple approximate formula for the quantum correction in the limit of the relativistic motion when the direction of the particle motion is parallel to that of the electric field.

  12. Design of model experiments for melt flow and solidification in a square container under time-dependent magnetic fields

    NASA Astrophysics Data System (ADS)

    Meier, D.; Lukin, G.; Thieme, N.; Bönisch, P.; Dadzis, K.; Büttner, L.; Pätzold, O.; Czarske, J.; Stelter, M.

    2017-03-01

    This paper describes novel equipment for model experiments designed for detailed studies on electromagnetically driven flows as well as solidification and melting processes with low-melting metals in a square-based container. Such model experiments are relevant for a validation of numerical flow simulation, in particular in the field of directional solidification of multi-crystalline photovoltaic silicon ingots. The equipment includes two square-shaped electromagnetic coils and a melt container with a base of 220×220 mm2 and thermostat-controlled heat exchangers at top and bottom. A system for dual-plane, spatial- and time-resolved flow measurements as well as for in-situ tracking of the solid-liquid interface is developed on the basis of the ultrasound Doppler velocimetry. The parameters of the model experiment are chosen to meet the scaling laws for a transfer of experimental results to real silicon growth processes. The eutectic GaInSn alloy and elemental gallium with melting points of 10.5 °C and 29.8 °C, respectively, are used as model substances. Results of experiments for testing the equipment are presented and discussed.

  13. Non-linear optics and local-field factors in liquid chloroform: A time-dependent density-functional theory study

    NASA Astrophysics Data System (ADS)

    Strubbe, David A.; Andrade, Xavier; Rubio, Angel; Louie, Steve G.

    2009-03-01

    Chloroform is often used as a solvent and reference when measuring non-linear optical properties of organic molecules. We calculate directly the non-linear susceptibilities of liquid chloroform at optical frequencies, using molecular dynamics and the Sternheimer equation in time-dependent density-functional theory [X. Andrade et al., J. Chem. Phys. 126, 184106 (2007)]. We compare the results to those of chloroform in the gas and solid phases, and experimental values, and make an ab initio calculation of the local-field factors which are needed to extract molecular properties from liquid calculations and experimental measurements.

  14. Time Dependent Fluids

    ERIC Educational Resources Information Center

    Collyer, A. A.

    1974-01-01

    Discusses the flow characteristics of thixotropic and negative thixotropic fluids; various theories underlying the thixotropic behavior; and thixotropic phenomena exhibited in drilling muds, commercial paints, pastes, and greases. Inconsistencies in the terminology used to label time dependent effects are revealed. (CC)

  15. Development of an efficient computer code to solve the time-dependent Navier-Stokes equations. [for predicting viscous flow fields about lifting bodies

    NASA Technical Reports Server (NTRS)

    Harp, J. L., Jr.; Oatway, T. P.

    1975-01-01

    A research effort was conducted with the goal of reducing computer time of a Navier Stokes Computer Code for prediction of viscous flow fields about lifting bodies. A two-dimensional, time-dependent, laminar, transonic computer code (STOKES) was modified to incorporate a non-uniform timestep procedure. The non-uniform time-step requires updating of a zone only as often as required by its own stability criteria or that of its immediate neighbors. In the uniform timestep scheme each zone is updated as often as required by the least stable zone of the finite difference mesh. Because of less frequent update of program variables it was expected that the nonuniform timestep would result in a reduction of execution time by a factor of five to ten. Available funding was exhausted prior to successful demonstration of the benefits to be derived from the non-uniform time-step method.

  16. An alternative approach to exact wave functions for time-dependent coupled oscillator model of charged particle in variable magnetic field

    SciTech Connect

    Menouar, Salah; Maamache, Mustapha; Choi, Jeong Ryeol

    2010-08-15

    The quantum states of time-dependent coupled oscillator model for charged particles subjected to variable magnetic field are investigated using the invariant operator methods. To do this, we have taken advantage of an alternative method, so-called unitary transformation approach, available in the framework of quantum mechanics, as well as a generalized canonical transformation method in the classical regime. The transformed quantum Hamiltonian is obtained using suitable unitary operators and is represented in terms of two independent harmonic oscillators which have the same frequencies as that of the classically transformed one. Starting from the wave functions in the transformed system, we have derived the full wave functions in the original system with the help of the unitary operators. One can easily take a complete description of how the charged particle behaves under the given Hamiltonian by taking advantage of these analytical wave functions.

  17. Time-Dependent Deformation at Brady Hot Springs Geothermal Field (Nevada) Measured With Interferometric Synthetic Aperture Radar and Modeled with Multiple Working Hypotheses of Coupled Behavior

    NASA Astrophysics Data System (ADS)

    Feigl, K. L.; Ali, S. T.; Akerley, J.; Baluyut, E.; Cardiff, M. A.; Davatzes, N. C.; Foxall, W.; Fratta, D.; Kreemer, C.; Mellors, R. J.; Lopeman, J.; Spielman, P.; Wang, H. F.

    2015-12-01

    To measure time-dependent deformation at the Brady Hot Springs geothermal field in western Nevada, we analyze interferometric synthetic aperture radar (InSAR) data acquired between 2004 and 2014 by five satellite missions, including: ERS-2, Envisat, ALOS, TerraSAR-X, and TanDEM-X. The resulting maps of deformation show an elliptical subsiding area that is ~4 km by ~1.5 km. Its long axis coincides with the strike of the dominant normal-fault system at Brady. Within this bowl of subsidence, the interference pattern shows several smaller features with length scales of the order of ~1 km. This signature occurs consistently in all of the well-correlated interferometric pairs spanning several months. Results from inverse modeling suggest that the deformation is a result of volumetric contraction in shallow units, no deeper than 600 m, that are probably associated with damaged regions where faults interact via thermal (T), hydrological (H), mechanical (M), and chemical (C) processes. Such damaged zones are expected to extend downward along steeply dipping fault planes, providing high-permeability conduits to the production wells. Using time series analysis, we test the hypothesis that geothermal production drives the observed deformation. We find a good correlation between the observed deformation rate and the rate of production in the shallow wells. We explore first-order models to calculate the time-dependent deformation fields produced by coupled processes, including: thermal contraction of rock (T-M coupling), decline in pore pressure (H-M coupling), and dissolution of minerals over time (H-C-M coupling). These processes are related to the heterogeneity of hydro-geological and material properties at the site. This work is part of a project entitled "Poroelastic Tomography by Adjoint Inverse Modeling of Data from Seismology, Geodesy, and Hydrology" (PoroTomo) http://geoscience.wisc.edu/feigl/porotomo.

  18. Off-equilibrium scaling behaviors driven by time-dependent external fields in three-dimensional O(N) vector models.

    PubMed

    Pelissetto, Andrea; Vicari, Ettore

    2016-03-01

    We consider the dynamical off-equilibrium behavior of the three-dimensional O(N) vector model in the presence of a slowly varying time-dependent spatially uniform magnetic field H(t)=h(t)e, where e is an N-dimensional constant unit vector, h(t)=t/t(s), and t(s) is a time scale, at fixed temperature T≤T(c), where T(c) corresponds to the continuous order-disorder transition. The dynamic evolutions start from equilibrium configurations at h(i)<0, correspondingly t(i)<0, and end at time t(f)>0 with h(t(f))>0, or vice versa. We show that the magnetization displays an off-equilibrium scaling behavior close to the transition line H(t)=0. It arises from the interplay among the time t, the time scale t(s), and the finite size L. The scaling behavior can be parametrized in terms of the scaling variables t(s)(κ)/L and t/t(s)(κ(t)), where κ>0 and κ(t)>0 are appropriate universal exponents, which differ at the critical point and for Ttime dependence of the external field. We define a scaling function for the hysteresis loop area of the magnetization that can be used to quantify how far the system is from equilibrium.

  19. Apparatus for performing oil field laser operations

    DOEpatents

    Zediker, Mark S.; Land, Mark S.; Rinzler, Charles C.; Faircloth, Brian O.; Koblick, Yeshaya; Moxley, Joel F.

    2017-01-03

    A system, apparatus and methods for delivering high power laser energy to perform laser operations in oil fields and to form a borehole deep into the earth using laser energy. A laser downhole assembly for the delivery of high power laser energy to surfaces and areas in a borehole, which assembly may have laser optics and a fluid path.

  20. The effect of the time dependent angular distribution of the intergrain magnetic field on the transport critical current in Ag-(Bi,Pb)2Sr2Ca2Cu3Ox tapes

    NASA Astrophysics Data System (ADS)

    Glowacki, B. A.; Noji, H.; Oota, A.

    1996-08-01

    Changes in the energy dissipation of the tape form Ag-(Bi,Pb)2Sr2Ca2Cu3Ox conductor have been interpreted in terms of magnetic flux movement from, or into, the intergrain regions of the highly textured plate like grain structure. The time dependent increase or decrease of the transport critical current (Ic), originates from time dependent angular superposition of the current induced self field (HSF), and external magnetic field [field cooling (HFC), and zero-field cooling (HZFC)] at the intergrain regions. The existence of time dependent changes of Ic can be explained in terms of the time dependent flux redistribution in grains and grain boundaries caused by thermal relaxation processes.

  1. 'Self-consistent' production of ion conics on return current region auroral field lines - A time-dependent, semi-kinetic model

    NASA Technical Reports Server (NTRS)

    Brown, David G.; Wilson, Gordon R.; Horwitz, James L.; Gallagher, Dennis L.

    1991-01-01

    We describe initial results from a time-dependent, semi-kinetic model of plasma outflow incorporating wave-particle interactions along current-carrying auroral field lines. Electrostatic waves are generated by the current driven ion cyclotron instability (CDICI), causing perpendicular velocity diffusion of ions plus electron heating via anomalous resistivity when and where the relative drift between electrons and ions exceeds certain critical velocities. Using the local bulk parameters we calculate these critical velocities, and so are able to self-consistently switch on and off the heating of the various particle species. Due to the dependence of these critical velocities on the bulk parameters of the species the heating effects exhibit quite complex spatial and temporal variations. A wide range of ion distribution functions are observed in these simulations, including conics with energies of a few electron volts and 'ring' distributions. The rings are seen to be a natural result of transverse heating and velocity filter effects and do not require coherent acceleration processes. We also observe the formation of a density depletion in hydrogen and enhanced oxygen densities at high altitudes.

  2. Time-dependent wellbore breakout growth caused by drilling-induced pore pressure transients: Implications for estimations of far field stress magnitude

    NASA Astrophysics Data System (ADS)

    Olcott, K. A.; Saffer, D. M.; Elsworth, D.

    2013-12-01

    One method used to constrain principal stress orientations and magnitudes in the crust combines estimates of rock strength with observations of wellbore failures, including drilling-induced tensile fractures (DITF) and compressional borehole breakouts (BO). This method has been applied at numerous Integrated Ocean Drilling Program (IODP) boreholes drilled into sediments in a wide range of settings, including the Gulf of Mexico, the N. Japan and Costa Rican subduction margins, and the Nankai Trough Accretionary Prism. At Nankai and N. Japan, BO widths defined by logging-while-drilling (LWD) resistivity images have been used to estimate magnitudes of far-field horizontal tectonic stresses. At several drillsites (C0010, C0002, and C0011), sections of the borehole were relogged with LWD after the hole was left open for times ranging from ~30 min to 3 days; times between acquisition were associated with pipe connections (~30 min), cleaning and circulating the hole (up to ~3 hr), and evacuation of the site for weather (~3 days). Relogged portions exhibit widening of BO, hypothesized to reflect time-dependent re-equilibration of instantaneous changes in pore fluid pressure (Pf) induced by opening the borehole. In this conceptual model, Pf decrease caused by initial excavation of the borehole and resulting changes in the state of stress at the borehole wall lead to an initial strengthening of the sediment. Re-equilibration of Pf results in time-dependent weakening of the sediment and subsequent BO growth. If correct, this hypothesis implies that stress magnitudes estimated by BO widths could be significantly underestimated. We test this idea using a finite-element model in COMSOL multiphysics that couples fluid flow and deformation in a poroelastic medium. We specify far-field horizontal principal stresses (SHmax and Shmin) in the model domain. At the start of simulations/at the time of borehole opening, we impose a decreased stress at the borehole wall. We consider a

  3. Laser intensity determination using nonadiabatic tunneling ionization of atoms in close-to-circularly polarized laser fields.

    PubMed

    Quan, Wei; Yuan, MingHu; Yu, ShaoGang; Xu, SongPo; Chen, YongJu; Wang, YanLan; Sun, RenPing; Xiao, ZhiLei; Gong, Cheng; Hua, LinQiang; Lai, XuanYang; Liu, XiaoJun; Chen, Jing

    2016-10-03

    We conceive an improved procedure to determine the laser intensity with the momentum distributions from nonadiabatic tunneling ionization of atoms in the close-to-circularly polarized laser fields. The measurements for several noble gas atoms are in accordance with the semiclassical calculations, where the nonadiabatic effect and the influence of Coulomb potential are included. Furthermore, the high-order above-threshold ionization spectrum in linearly polarized laser fields for Ar is measured and compared with the numerical calculation of the time-dependent Schrödinger equation in the single-active-electron approximation to test the accuracy of the calibrated laser intensity.

  4. Time-Dependent Photodissociation Regions

    NASA Technical Reports Server (NTRS)

    Hollenbach, David; Natta, Antonella

    1995-01-01

    We present theoretical models of the time-dependent thermal and chemical structure of molecular gas suddenly exposed to far-ultraviolet (FUV) (6 eV less than hv less than 13.6 eV) radiation fields and the consequent time- dependent infrared emission of the gas. We focus on the response of molecular hydrogen for cloud densities ranging from n = 10(exp 3) to 10(exp 6)/cu cm and FUV fluxes G(sub 0) = 10(exp 3)-10(exp 6) times the local FUV interstellar flux. For G(sub 0)/n greater than 10(exp -2) cu cm, the emergent H(sub 2) vibrational line intensities are initially larger than the final equilibrium values. The H(sub 2) lines are excited by FUV fluorescence and by collisional excitation in warm gas. Most of the H(sub 2) intensity is generated at a characteristic hydrogen column density of N approximately 10(exp 21)/sq cm, which corresponds to an FUV optical depth of unity caused by dust opacity. The time dependence of the H(sub 2) intensities arises because the initial abundances of H(sub 2) at these depths is much higher than the equilibrium values, so that H(sub 2) initially competes more effectively with dust in absorbing FUV photons. Considerable column densities of warm (T approximately 1000) K H(sub 2) gas can be produced by the FUV pumping of H(sub 2) vibrational levels followed by collisional de-excitation, which transfers the energy to heat. In dense (n greater than or approximately 10(exp 5)/cu cm) gas exposed to high (G(sub 0) greater than or approximately 10(exp 4)) fluxes, this warm gas produces a 2-1 S(1)/1-0 S(l) H(sub 2) line ratio of approximately 0.1, which mimics the ratio found in shocked gas. In lower density regions, the FUV pumping produces a pure-fluorescent ratio of approximately 0.5. We also present calculations of the time dependence of the atomic hydrogen column densities and of the intensities of 0 I 6300 A, S II 6730 A, Fe II 1.64 microns, and rotational OH and H20 emission. Potential applications include star-forming regions, clouds

  5. Birefringence in time-dependent moving media

    NASA Astrophysics Data System (ADS)

    Lin, Shirong; Zhang, Ruoyang; Zhai, Yanwang; Wei, Jianye; Zhao, Qing

    2016-08-01

    Electromagnetic wave propagation in one- and two-dimensional time-dependent moving media is investigated in this paper. We identify another origin of linear birefringence caused by the component of the flow perpendicular to the wave vector. Previously, birefringence is induced by applying external electric and magnetic fields to non-crystalline material. Here it is shown that the time-varying velocity field also contributes to such a phenomenon. Our results indicate that the parallel component, time-dependent or not, will not yield birefringence. Furthermore, the time-dependent flow also results in a frequency shift. One-dimensional simulation is conducted to demonstrate these effects.

  6. Determination of efficiencies, loss mechanisms, and performance degradation factors in chopper controlled dc vehical motors. Section 2: The time dependent finite element modeling of the electromagnetic field in electrical machines: Methods and applications. Ph.D. Thesis

    NASA Technical Reports Server (NTRS)

    Hamilton, H. B.; Strangas, E.

    1980-01-01

    The time dependent solution of the magnetic field is introduced as a method for accounting for the variation, in time, of the machine parameters in predicting and analyzing the performance of the electrical machines. The method of time dependent finite element was used in combination with an also time dependent construction of a grid for the air gap region. The Maxwell stress tensor was used to calculate the airgap torque from the magnetic vector potential distribution. Incremental inductances were defined and calculated as functions of time, depending on eddy currents and saturation. The currents in all the machine circuits were calculated in the time domain based on these inductances, which were continuously updated. The method was applied to a chopper controlled DC series motor used for electric vehicle drive, and to a salient pole sychronous motor with damper bars. Simulation results were compared to experimentally obtained ones.

  7. Spatiotemporal distribution of strain field and hydraulic conductivity at the Phoenix valley basins, constrained using InSAR time series and time-dependent models

    NASA Astrophysics Data System (ADS)

    Miller, M. M.; Shirzaei, M.

    2015-12-01

    Poroelastic theory suggests that long-term aquifer deformation is linearly proportional to changes in pore pressure. Land subsidence is the surface expression of deformation occurring at depth that is observed with dense, detailed, and high precision interferometric SAR data. In earlier work, Miller & Shirzaei [2015] identified zones of subsidence and uplift across the Phoenix valley caused by pumping and artificial recharge operations. we combined ascending and descending Envisat InSAR datasets to estimate vertical and horizontal displacement time series from 2003-2010. Next, wavelet decomposition was used to extract and compare the elastic components of vertical deformation and hydraulic head data to estimate aquifer storage coefficients. In the following, we present the results from elastic aquifer modeling using a 3D array of triangular dislocations, extending from depth of 0.5 to 3.5 km. We employ a time-dependent modeling scheme to invert the InSAR displacement time series, solving for the spatiotemporal distribution of the aquifer-aquitard compaction. Such models are used to calculate strain and stress fields and forecast the location of extensional cracks and earth fissures, useful for urban planning and management. Later, applying the framework suggested by Burbey [1999], the optimum compaction model is used to estimate the 3D distribution of hydraulic conductivities as a function of time. These estimates are verified using in-situ and laboratory observations and provide unique evidence to investigate the stress-dependence of the hydraulic conductivity and its variations due to pumping, recharge, and injection. The estimates will also be used in groundwater flow models, enhancing water management in the valley and elsewhere. References Burby, T. J. (1999), Effects of horizontal strain in estimating specific storage and compaction in confined and leaky aquifer systems, Hydrogeology Journal, 7(6), 521-532, doi:10.1007/s100400050225

  8. The dynamics of small molecules in intense laser fields

    NASA Astrophysics Data System (ADS)

    Posthumus, J. H.

    2004-05-01

    In the past decade, the understanding of the dynamics of small molecules in intense laser fields has advanced enormously. At the same time, the technology of ultra-short pulsed lasers has equally progressed to such an extent that femtosecond lasers are now widely available. This review is written from an experimentalist's point of view and begins by discussing the value of this research and defining the meaning of the word 'intense'. It continues with describing the Ti : sapphire laser, including topics such as pulse compression, chirped pulse amplification, optical parametric amplification, laser-pulse diagnostics and the absolute phase. Further aspects include focusing, the focal volume effect and space charge. The discussion of physics begins with the Keldysh parameter and the three regimes of ionization, i.e. multi-photon, tunnelling and over-the-barrier. Direct-double ionization (non-sequential ionization), high-harmonic generation, above-threshold ionization and attosecond pulses are briefly mentioned. Subsequently, a theoretical calculation, which solves the time-dependent Schrödinger equation, is compared with an experimental result. The dynamics of H_{2}^{ + } in an intense laser field is interpreted in terms of bond-softening, vibrational trapping (bond-hardening), below-threshold dissociation and laser-induced alignment of the molecular axis. The final section discusses the modified Franck-Condon principle, enhanced ionization at critical distances and Coulomb explosion of diatomic and triatomic molecules.

  9. Time dependent Doppler shifts in high-order harmonic generation in intense laser interactions with solid density plasma and frequency chirped pulses

    SciTech Connect

    Welch, E. C.; Zhang, P.; He, Z.-H.; Dollar, F.; Krushelnick, K.; Thomas, A. G. R.

    2015-05-15

    High order harmonic generation from solid targets is a compelling route to generating intense attosecond or even zeptosecond pulses. However, the effects of ion motion on the generation of harmonics have only recently started to be considered. Here, we study the effects of ion motion in harmonics production at ultrahigh laser intensities interacting with solid density plasma. Using particle-in-cell simulations, we find that there is an optimum density for harmonic production that depends on laser intensity, which scales linearly with a{sub 0} with no ion motion but with a reduced scaling if ion motion is included. We derive a scaling for this optimum density with ion motion and also find that the background ion motion induces Doppler red-shifts in the harmonic structures of the reflected pulse. The temporal structure of the Doppler shifts is correlated to the envelope of the incident laser pulse. We demonstrate that by introducing a frequency chirp in the incident pulse we are able to eliminate these Doppler shifts almost completely.

  10. Photoassociation of cold atoms with chirped laser pulses: Time-dependent calculations and analysis of the adiabatic transfer within a two-state model

    SciTech Connect

    Luc-Koenig, E.; Masnou-Seeuws, F.; Kosloff, R.; Vatasescu, M.

    2004-09-01

    This theoretical paper presents numerical calculations for the photoassociation of ultracold cesium atoms with a chirped laser pulse and a detailed analysis of the results. In contrast with earlier work, the initial state is represented by a stationary continuum wave function. In the chosen example, it is shown that an important population transfer is achieved to {approx_equal}15 vibrational levels in the vicinity of the v=98 bound level in the external well of the 0{sub g}{sup -}(6s+6p{sub 3/2}) potential. Such levels lie in the energy range swept by the instantaneous frequency of the pulse, thus defining a 'photoassociation window'. Levels outside this window may be significantly excited during the pulse, but no population remains there after the pulse. Finally, the population transfer to the last vibrational levels of the ground a {sup 3}{sigma}{sub u}{sup +}(6s+6s) state is significant, making stable molecules. The results are interpreted in the framework of a two-state model as an adiabatic inversion mechanism, efficient only within the photoassociation window. The large value found for the photoassociation rate suggests promising applications. The present chirp has been designed in view of creating in the excited state a vibrational wave packet that is focusing at the barrier of the double-well potential.

  11. Effect of external and internal magnetic fields on the bias stability in a Zeeman laser gyroscope

    SciTech Connect

    Kolbas, Yu Yu; Saveliev, I I; Khokhlov, N I

    2015-06-30

    With the specific features of electronic systems of a Zeeman laser gyroscope taken into account, the basic physical mechanisms of the magnetic field effect on the bias stability and the factors giving rise to the internal magnetic fields are revealed. The hardware-based methods of reducing the effect of external and internal magnetic fields are considered, as well as the algorithmic methods for increasing the stability of the bias magnetic component by taking into account its reproducible temperature and time dependences. Typical experimental temperature and time dependences of the magnetic component of the Zeeman laser gyro bias are presented, and by their example the efficiency of the proposed methods for reducing the effect of magnetic fields is shown. (laser gyroscopes)

  12. Long-time solution of the time-dependent Schroedinger equation for an atom in an electromagnetic field using complex coordinate contours

    SciTech Connect

    Tao, Liang; Vanroose, Wim; Reps, Brian; Rescigno, Thomas N.; McCurdy, C. William

    2009-09-08

    We demonstrate that exterior complex scaling (ECS) can be used to impose outgoing wave boundary conditions exactly on solutions of the time-dependent Schrodinger equation for atoms in intense electromagnetic pulses using finite grid methods. The procedure is formally exact when applied in the appropriate gauge and is demonstrated in a calculation of high harmonic generation in which multiphoton resonances are seen for long pulse durations. However, we also demonstrate that while the application of ECS in this way is formally exact, numerical error can appear for long time propagations that can only be controlled by extending the finite grid. A mathematical analysis of the origins of that numerical error, illustrated with an analytically solvable model, is also given.

  13. Role of enhanced laser field in laser processing of nanomaterials

    NASA Astrophysics Data System (ADS)

    Zhang, Tao; Kuk, Seungkuk; Kim, Eunpa; Grigoropoulos, Costas P.; Hwang, David J.

    2016-03-01

    Lasers have proven to be unique tools for a highly selective processing of nanomaterials system on the basis of the enhanced laser field, maintaining other sensitive portion in the system untouched. However, in many practical applications, a wide interspacing distribution among nanomaterials and nonlinear laser absorption properties of the nanomaterials in the highly excited nanomaterials states, frequently lead to rather adverse effects in terms of controlled nanomaterials processing. In this study, we will take a few laser nanomaterials processing examples mainly based on the nanowires system including the spin coated metallic nanowires for transparent electrode applications and selective semiconductor nanowires growth from the metallic nanocatalysts, and discuss on the role of the enhanced laser field via the combined theoretical and experimental investigations. Specific aims of properly utilizing the enhanced laser fields are to achieve improved electrical conductance for practical transparent electrode applications, and to facilitate directed growth of semiconductor nanowires at designated sample locations, respectively.

  14. Laser Resurfacing: Full Field and Fractional.

    PubMed

    Pozner, Jason N; DiBernardo, Barry E

    2016-07-01

    Laser resurfacing is a very popular procedure worldwide. Full field and fractional lasers are used in many aesthetic practices. There have been significant advances in laser resurfacing in the past few years, which make patient treatments more efficacious and with less downtime. Erbium and carbon dioxide and ablative, nonablative, and hybrid fractional lasers are all extremely effective and popular tools that have a place in plastic surgery and dermatology offices.

  15. Offset angles of photocurrents generated in few-cycle circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Liu, Jinlei; Fu, Yongsheng; Chen, Wenbo; Lü, Zhihui; Zhao, Jing; Yuan, Jianmin; Zhao, Zengxiu

    2017-03-01

    Photocurrents generated in few-cycle circularly polarized laser fields are investigated by solving the time-dependent Schrödinger equation and by means of classical-trajectory Monte Carlo simulations. After confirming the offset angles of the total final currents and electron spectra to be the same, we illustrate the effects of the Coulomb potential and ground state depletion on the offset angles of the total final current, by analyzing how electrons’ trajectories and momenta change with laser intensities. Using various atom systems at different laser wavelengths, we find that the behaviors of currents’ offset angles as a function of laser intensities seem to be universal.

  16. Time-dependent wave front propagation simulation of a hard x-ray split-and-delay unit: Towards a measurement of the temporal coherence properties of x-ray free electron lasers

    DOE PAGES

    Roling, S.; Zacharias, H.; Samoylova, L.; ...

    2014-11-18

    For the European x-ray free electron laser (XFEL) a split-and-delay unit based on geometrical wavefront beam splitting and multilayer mirrors is built which covers the range of photon energies from 5 keV up to 20 keV. Maximum delays between Δτ = ±2.5 ps at hν=20 keV and up to Δτ = ±23 ps at hν = 5 keV will be possible. Time-dependent wave-optics simulations have been performed by means of Synchrotron Radiation Workshop software for XFEL pulses at hν = 5 keV. The XFEL radiation was simulated using results of time-dependent simulations applying the self-amplified spontaneous emission code FAST. Mainmore » features of the optical layout, including diffraction on the beam splitter edge and optics imperfections measured with a nanometer optic component measuring machine slope measuring profiler, were taken into account. The impact of these effects on the characterization of the temporal properties of XFEL pulses is analyzed. An approach based on fast Fourier transformation allows for the evaluation of the temporal coherence despite large wavefront distortions caused by the optics imperfections. In this manner, the fringes resulting from time-dependent two-beam interference can be filtered and evaluated yielding a coherence time of τc = 0.187 fs (HWHM) for real, nonperfect mirrors, while for ideal mirrors a coherence time of τc = 0.191 fs (HWHM) is expected.« less

  17. Time-dependent wave front propagation simulation of a hard x-ray split-and-delay unit: Towards a measurement of the temporal coherence properties of x-ray free electron lasers

    SciTech Connect

    Roling, S.; Zacharias, H.; Samoylova, L.; Sinn, H.; Tschentscher, Th.; Chubar, O.; Buzmakov, A.; Schneidmiller, E.; Yurkov, M. V.; Siewert, F.; Braun, S.; Gawlitza, P.

    2014-11-18

    For the European x-ray free electron laser (XFEL) a split-and-delay unit based on geometrical wavefront beam splitting and multilayer mirrors is built which covers the range of photon energies from 5 keV up to 20 keV. Maximum delays between Δτ = ±2.5 ps at hν=20 keV and up to Δτ = ±23 ps at hν = 5 keV will be possible. Time-dependent wave-optics simulations have been performed by means of Synchrotron Radiation Workshop software for XFEL pulses at hν = 5 keV. The XFEL radiation was simulated using results of time-dependent simulations applying the self-amplified spontaneous emission code FAST. Main features of the optical layout, including diffraction on the beam splitter edge and optics imperfections measured with a nanometer optic component measuring machine slope measuring profiler, were taken into account. The impact of these effects on the characterization of the temporal properties of XFEL pulses is analyzed. An approach based on fast Fourier transformation allows for the evaluation of the temporal coherence despite large wavefront distortions caused by the optics imperfections. In this manner, the fringes resulting from time-dependent two-beam interference can be filtered and evaluated yielding a coherence time of τc = 0.187 fs (HWHM) for real, nonperfect mirrors, while for ideal mirrors a coherence time of τc = 0.191 fs (HWHM) is expected.

  18. Investigations of Low Temperature Time Dependent Cracking

    SciTech Connect

    Van der Sluys, W A; Robitz, E S; Young, B A; Bloom, J

    2002-09-30

    The objective of this project was to investigate metallurgical and mechanical phenomena associated with time dependent cracking of cold bent carbon steel piping at temperatures between 327 C and 360 C. Boiler piping failures have demonstrated that understanding the fundamental metallurgical and mechanical parameters controlling these failures is insufficient to eliminate it from the field. The results of the project consisted of the development of a testing methodology to reproduce low temperature time dependent cracking in laboratory specimens. This methodology was used to evaluate the cracking resistance of candidate heats in order to identify the factors that enhance cracking sensitivity. The resultant data was integrated into current available life prediction tools.

  19. Influence of time dependent longitudinal magnetic fields on the cooling process, exchange bias and magnetization reversal mechanism in FM core/AFM shell nanoparticles: a Monte Carlo study

    NASA Astrophysics Data System (ADS)

    Yüksel, Yusuf; Akıncı, Ümit

    2016-12-01

    Using Monte Carlo simulations, we have investigated the dynamic phase transition properties of magnetic nanoparticles with ferromagnetic core coated by an antiferromagnetic shell structure. Effects of field amplitude and frequency on the thermal dependence of magnetizations, magnetization reversal mechanisms during hysteresis cycles, as well as on the exchange bias and coercive fields have been examined, and the feasibility of applying dynamic magnetic fields on the particle have been discussed for technological and biomedical purposes.

  20. Enhancement of terahertz radiation by using circularly polarized two-color laser fields

    NASA Astrophysics Data System (ADS)

    Meng, Chao; Chen, Wenbo; Wang, Xiaowei; Lü, Zhihui; Huang, Yindong; Liu, Jinlei; Zhang, Dongwen; Zhao, Zengxiu; Yuan, Jianmin

    2016-09-01

    Terahertz radiation from tunneling ionization of gaseous atoms and molecules in the two-color laser fields with various polarizations has been investigated. We experimentally demonstrate that the efficiency of terahertz emission in the circularly polarized laser fields with the same helicity is 5 times higher than that with linearly polarized two-color femtosecond pulses in high laser intensity. By solving time-dependent Schrödinger equation, this enhancement is well explained based on the analysis of electron tunneling ionization and subsequent dynamics.

  1. EUV two-photon-ionization cross sections of helium from the solution of the time-dependent Schrödinger equation, and comparison with measurements using free-electron lasers

    NASA Astrophysics Data System (ADS)

    Mercouris, Theodoros; Komninos, Yannis; Nicolaides, Cleanthes A.

    2016-12-01

    Two recent experimental papers reported the first measurements of absolute two-photon-ionization cross sections σ (2 ) of helium, for EUV wavelengths, using free-electron laser (FEL) pulses [Sato et al., J. Phys. B 44, 161001 (2011), 10.1088/0953-4075/44/16/161001; Fushitani et al., Phys. Rev. A 88, 063422 (2013), 10.1103/PhysRevA.88.063422]. The wavelengths correspond to transitions that are off resonance as well as on resonance with the 1 s 2 p and 1 s 3 p 1Po Rydberg states. Inspection of their results reveals considerable discrepancies, while their comparison with theoretical results obtained earlier from time-independent calculations, one perturbative and two nonperturbative ones, cannot lead to secure conclusions as to the true values of σ (2 ) . We examined this prototypical problem by implementing a time-dependent approach, which utilizes the nonperturbative solution of the time-dependent Schrödinger equation. This solution was obtained in terms of the state-specific expansion approach, in an upgraded version where the coupling matrix elements are computed using the full electric operator of the multipolar Hamiltonian. The σ (2 ) were obtained for pulses of 300 fs, as in the 2011 FEL experiment. Their computation was achieved by fitting the time-dependent ionization survival probability to e-Γ t, where Γ is the rate of ionization. The wavelengths and intensities are those of the FEL experiments, as well as others, such as the wavelengths 52.22 and 51.56 nm, for which the 1 s 4 p 1Po and 1 s 5 p 1Po levels are on resonance with the initial 1S state. Apart from the predictions for these wavelengths, the paper contains characteristic comparisons among all the results on these EUV σ (2 ) , experimental and theoretical. In general, the trends predicted by nonperturbative methods are confirmed by the FEL measurements. However, discrepancies exist among the absolute numbers. Furthermore, comparison among the results of the three nonperturbative approaches

  2. Strong-Field Control of Laser Filamentation Mechanisms

    NASA Astrophysics Data System (ADS)

    Levis, Robert; Romanov, Dmitri; Filin, Aleskey; Compton, Ryan

    2008-05-01

    The propagation of short strong-file laser pulses in gas and solution phases often result in formation of filaments. This phenomenon involves many nonlinear processes including Kerr lensing, group velocity dispersion, multi-photon ionization, plasma defocusing, intensity clamping, and self-steepening. Of these, formation and dynamics of pencil-shape plasma areas plays a crucial role. The fundamental understanding of these laser-induced plasmas requires additional effort, because the process is highly nonlinear and complex. We studied the ultrafast laser-generated plasma dynamics both experimentally and theoretically. Ultrafast plasma dynamics was probed using Coherent Anti-Stokes Raman Scattering. The measurements were made in a room temperature gas maintained at 1 atm in a flowing cell. The time dependent scattering was measured by delaying the CARS probe with respect to the intense laser excitation pulse. A general trend is observed between the spacing of the ground state and the first allowed excited state with the rise time for the noble gas series and the molecular gases. This trend is consistent with our theoretical model, which considers the ultrafast dynamics of the strong field generated plasma as a three-step process; (i) strong-field ionization followed by the electron gaining considerable kinetic energy during the pulse; (ii) immediate post-pulse dynamics: fast thermalization, impact-ionization-driven electron multiplication and cooling; (iii) ensuing relaxation: evolution to electron-ion equilibrium and eventual recombination.

  3. Dynamic phase transition properties and hysteretic behavior of a ferrimagnetic core-shell nanoparticle in the presence of a time dependent magnetic field

    NASA Astrophysics Data System (ADS)

    Yüksel, Yusuf; Vatansever, Erol; Polat, Hamza

    2012-10-01

    We have presented dynamic phase transition features and stationary-state behavior of a ferrimagnetic small nanoparticle system with a core-shell structure. By means of detailed Monte Carlo simulations, a complete picture of the phase diagrams and magnetization profiles has been presented and the conditions for the occurrence of a compensation point Tcomp in the system have been investigated. According to Néel nomenclature, the magnetization curves of the particle have been found to obey P-type, N-type and Q-type classification schemes under certain conditions. Much effort has been devoted to investigating the hysteretic response of the particle, and we observed the existence of triple hysteresis loop behavior, which originates from the existence of a weak ferromagnetic core coupling Jc/Jsh, as well as a strong antiferromagnetic interface exchange interaction Jint/Jsh. Most of the calculations have been performed for a particle in the presence of oscillating fields of very high frequencies and high amplitudes in comparison with exchange interactions, which resembles a magnetic system under the influence of ultrafast switching fields. Particular attention has also been paid to the influence of the particle size on the thermal and magnetic properties, as well as magnetic features such as coercivity, remanence and the compensation temperature of the particle. We have found that, in the presence of ultrafast switching fields, the particle may exhibit a dynamic phase transition from paramagnetic to a dynamically ordered phase with increasing ferromagnetic shell thickness.

  4. Field-aligned currents in Saturn's magnetosphere: Local time dependence of southern summer currents in the dawn sector between midnight and noon

    NASA Astrophysics Data System (ADS)

    Hunt, G. J.; Cowley, S. W. H.; Provan, G.; Bunce, E. J.; Alexeev, I. I.; Belenkaya, E. S.; Kalegaev, V. V.; Dougherty, M. K.; Coates, A. J.

    2016-08-01

    We examine and compare the magnetic field perturbations associated with field-aligned ionosphere-magnetosphere coupling currents at Saturn, observed by the Cassini spacecraft during two sequences of highly inclined orbits in 2006/2007 and 2008 under late southern summer conditions. These sequences explore the southern currents in the dawn-noon and midnight sectors, respectively, thus allowing investigation of possible origins of the local time (LT) asymmetry in auroral Saturn kilometric radiation (SKR) emissions, which peak in power at ~8 h LT in the dawn-noon sector. We first show that the dawn-noon field data generally have the same four-sheet current structure as found previously in the midnight data and that both are similarly modulated by "planetary period oscillation" (PPO) currents. We then separate the averaged PPO-independent (e.g., subcorotation) and PPO-related currents for both LT sectors by using the current system symmetry properties. Surprisingly, we find that the PPO-independent currents are essentially identical within uncertainties in the dawn-dusk and midnight sectors, thus providing no explanation for the LT dependence of the SKR emissions. The main PPO-related currents are, however, found to be slightly stronger and narrower in latitudinal width at dawn-noon than at midnight, leading to estimated precipitating electron powers, and hence emissions, that are on average a factor of ~1.3 larger at dawn-noon than at midnight, inadequate to account for the observed LT asymmetry in SKR power by a factor of ~2.7. Some other factors must also be involved, such as a LT asymmetry in the hot magnetospheric auroral source electron population.

  5. Exact time dependence of solutions to the time-dependent Schrödinger equation

    NASA Astrophysics Data System (ADS)

    Lohe, M. A.

    2009-01-01

    Solutions of the Schrödinger equation with an exact time dependence are derived as eigenfunctions of dynamical invariants which are constructed from time-independent operators using time-dependent unitary transformations. Exact solutions and a closed form expression for the corresponding time evolution operator are found for a wide range of time-dependent Hamiltonians in d dimensions, including non-Hermitean {\\cal PT} -symmetric Hamiltonians. Hamiltonians are constructed using time-dependent unitary spatial transformations comprising dilatations, translations and rotations and solutions are found in several forms: as eigenfunctions of a quadratic invariant, as coherent state eigenfunctions of boson operators, as plane wave solutions from which the general solution is obtained as an integral transform by means of the Fourier transform, and as distributional solutions for which the initial wavefunction is the Dirac δ-function. For the isotropic harmonic oscillator in d dimensions radial solutions are found which extend known results for d = 1, including Barut-Girardello and Perelomov coherent states (i.e., vector coherent states), which are shown to be related to eigenfunctions of the quadratic invariant by the ζ-transformation. This transformation, which leaves the Ermakov equation invariant, implements SU(1, 1) transformations on linear dynamical invariants. \\mathfrak{su}(1, 1) coherent states are derived also for the time-dependent linear potential. Exact solutions are found for Hamiltonians with electromagnetic interactions in which the time-dependent magnetic and electric fields are not necessarily spatially uniform. As an example, it is shown how to find exact solutions of the time-dependent Schrödinger equation for the Dirac magnetic monopole in the presence of time-dependent magnetic and electric fields of a specified form.

  6. Unified Time and Frequency Picture of Ultrafast Atomic Excitation in Strong Laser Fields.

    PubMed

    Zimmermann, H; Patchkovskii, S; Ivanov, M; Eichmann, U

    2017-01-06

    Excitation and ionization in strong laser fields lies at the heart of such diverse research directions as high-harmonic generation and spectroscopy, laser-induced diffraction imaging, emission of femtosecond electron bunches from nanotips, self-guiding, filamentation and mirrorless lasing during propagation of light in atmospheres. While extensive quantum mechanical and semiclassical calculations on strong-field ionization are well backed by sophisticated experiments, the existing scattered theoretical work aiming at a full quantitative understanding of strong-field excitation lacks experimental confirmation. Here we present experiments on strong-field excitation in both the tunneling and multiphoton regimes and their rigorous interpretation by time dependent Schrödinger equation calculations, which finally consolidates the seemingly opposing strong-field regimes with their complementary pictures. Most strikingly, we observe an unprecedented enhancement of excitation yields, which opens new possibilities in ultrafast strong-field control of Rydberg wave packet excitation and laser intensity characterization.

  7. Unified Time and Frequency Picture of Ultrafast Atomic Excitation in Strong Laser Fields

    NASA Astrophysics Data System (ADS)

    Zimmermann, H.; Patchkovskii, S.; Ivanov, M.; Eichmann, U.

    2017-01-01

    Excitation and ionization in strong laser fields lies at the heart of such diverse research directions as high-harmonic generation and spectroscopy, laser-induced diffraction imaging, emission of femtosecond electron bunches from nanotips, self-guiding, filamentation and mirrorless lasing during propagation of light in atmospheres. While extensive quantum mechanical and semiclassical calculations on strong-field ionization are well backed by sophisticated experiments, the existing scattered theoretical work aiming at a full quantitative understanding of strong-field excitation lacks experimental confirmation. Here we present experiments on strong-field excitation in both the tunneling and multiphoton regimes and their rigorous interpretation by time dependent Schrödinger equation calculations, which finally consolidates the seemingly opposing strong-field regimes with their complementary pictures. Most strikingly, we observe an unprecedented enhancement of excitation yields, which opens new possibilities in ultrafast strong-field control of Rydberg wave packet excitation and laser intensity characterization.

  8. Polarization dependence in inelastic scattering of electrons by hydrogen atoms in a circularly polarized laser field

    NASA Astrophysics Data System (ADS)

    Buică, Gabriela

    2017-01-01

    We theoretically study the influence of laser polarization in inelastic scattering of electrons by hydrogen atoms in the presence of a circularly polarized laser field in the domain of field strengths below 107 V/cm and high projectile energies. A semi-perturbative approach is used in which the interaction of the projectile electrons with the laser field is described by Gordon-Volkov wave functions, while the interaction of the hydrogen atom with the laser field is described by first-order time-dependent perturbation theory. A closed analytical solution is derived in laser-assisted inelastic electron-hydrogen scattering for the 1 s → nl excitation cross section which is valid for both circular and linear polarizations. For the excitation of the n=2 levels simple analytical expressions of differential cross section are derived for laser-assisted inelastic scattering in the perturbative domain, and the differential cross sections by the circularly and linearly polarized laser fields and their ratios for one- and two-photon absorption are calculated as a function of the scattering angle. Detailed numerical results for the angular dependence and the resonance structure of the differential cross sections are discussed for the 1 s → 4 l excitations of hydrogen in a circularly polarized laser field.

  9. Stabilization of circular Rydberg atoms by circularly polarized infrared laser fields

    SciTech Connect

    Askeland, S.; Soerngaard, S. A.; Nepstad, R.; Foerre, M.; Pilskog, I.

    2011-09-15

    The ionization dynamics of circular Rydberg states in strong circularly polarized infrared (800 nm) laser fields is studied by means of numerical simulations with the time-dependent Schroedinger equation. We find that at certain intensities, related to the radius of the Rydberg states, atomic stabilization sets in, and the ionization probability decreases as the intensity is further increased. Moreover, there is a strong dependence of the ionization probability on the rotational direction of the applied laser field, which can be understood from a simple classical analogy.

  10. Strong field laser control of photochemistry.

    PubMed

    Solá, Ignacio R; González-Vázquez, Jesús; de Nalda, Rebeca; Bañares, Luis

    2015-05-28

    Strong ultrashort laser pulses have opened new avenues for the manipulation of photochemical processes like photoisomerization or photodissociation. The presence of light intense enough to reshape the potential energy surfaces may steer the dynamics of both electrons and nuclei in new directions. A controlled laser pulse, precisely defined in terms of spectrum, time and intensity, is the essential tool in this type of approach to control chemical dynamics at a microscopic level. In this Perspective we examine the current strategies developed to achieve control of chemical processes with strong laser fields, as well as recent experimental advances that demonstrate that properties like the molecular absorption spectrum, the state lifetimes, the quantum yields and the velocity distributions in photodissociation processes can be controlled by the introduction of carefully designed strong laser fields.

  11. Laser ion source with solenoid field

    SciTech Connect

    Kanesue, Takeshi; Fuwa, Yasuhiro; Kondo, Kotaro; Okamura, Masahiro

    2014-11-12

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. In this study, the laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 1011, which was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.

  12. Laser ion source with solenoid field

    DOE PAGES

    Kanesue, Takeshi; Fuwa, Yasuhiro; Kondo, Kotaro; ...

    2014-11-12

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. In this study, the laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 1011, whichmore » was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.« less

  13. Laser ion source with solenoid field

    NASA Astrophysics Data System (ADS)

    Kanesue, Takeshi; Fuwa, Yasuhiro; Kondo, Kotaro; Okamura, Masahiro

    2014-11-01

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. The laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 1011, which was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.

  14. Electromagnetically induced transparency in modulated laser fields

    NASA Astrophysics Data System (ADS)

    Jiao, Yuechun; Yang, Zhiwei; Zhang, Hao; Zhang, Linjie; Raithel, Georg; Zhao, Jianming; Jia, Suotang

    2017-02-01

    We study electromagnetically induced transparency (EIT) in a room-temperature cesium vapor cell using wavelength-modulated probe laser light. In the utilized cascade level scheme, the probe laser drives the lower transition 6S {}1/2(F = 4) → 6P {}3/2 (F’ = 5), while the coupling laser drives the Rydberg transition 6P {}3/2 → 57S {}1/2. The probe laser has a fixed average frequency and is modulated at a frequency of a few kHz, with a variable modulation amplitude in the range of tens of MHz. The probe transmission is measured as a function of the detuning of the coupling laser from the Rydberg resonance. The first-harmonic demodulated EIT signal has two peaks that are, in the case of large modulation amplitude, separated by the peak-to-peak modulation amplitude of the probe laser times a scaling factor {λ }{{p}}/{λ }{{c}}, where {λ }{{p}} and {λ }{{c}} are the probe- and coupling-laser wavelengths. The scaling factor is due to Doppler shifts in the EIT geometry. Second-harmonic demodulated EIT signals, obtained with small modulation amplitudes, yield spectral lines that are much narrower than corresponding lines in the modulation-free EIT spectra. The resultant spectroscopic resolution enhancement is conducive to improved measurements of radio-frequency (RF) fields based on Rydberg-atom EIT, an approach in which the response of Rydberg atoms to RF fields is exploited to characterize RF fields. Here, we employ wavelength modulation spectroscopy to reduce the uncertainty of atom-based frequency and field measurement of an RF field in the VHF radio band.

  15. Solvable time-dependent models in quantum mechanics

    NASA Astrophysics Data System (ADS)

    Cordero-Soto, Ricardo J.

    In the traditional setting of quantum mechanics, the Hamiltonian operator does not depend on time. While some Schrodinger equations with time-dependent Hamiltonians have been solved, explicitly solvable cases are typically scarce. This thesis is a collection of papers in which this first author along with Suslov, Suazo, and Lopez, has worked on solving a series of Schrodinger equations with a time-dependent quadratic Hamiltonian that has applications in problems of quantum electrodynamics, lasers, quantum devices such as quantum dots, and external varying fields. In particular the author discusses a new completely integrable case of the time-dependent Schrodinger equation in Rn with variable coefficients for a modified oscillator, which is dual with respect to the time inversion to a model of the quantum oscillator considered by Meiler, Cordero-Soto, and Suslov. A second pair of dual Hamiltonians is found in the momentum representation. Our examples show that in mathematical physics and quantum mechanics a change in the direction of time may require a total change of the system dynamics in order to return the system back to its original quantum state. The author also considers several models of the damped oscillators in nonrelativistic quantum mechanics in a framework of a general approach to the dynamics of the time-dependent Schrodinger equation with variable quadratic Hamiltonians. The Green functions are explicitly found in terms of elementary functions and the corresponding gauge transformations are discussed. The factorization technique is applied to the case of a shifted harmonic oscillator. The time-evolution of the expectation values of the energy related operators is determined for two models of the quantum damped oscillators under consideration. The classical equations of motion for the damped oscillations are derived for the corresponding expectation values of the position operator. Finally, the author constructs integrals of motion for several models

  16. Time Dependent Nuclear Scattering Calculations

    NASA Astrophysics Data System (ADS)

    Weeks, David

    2005-04-01

    A new time dependent method for calculating scattering matrix elements of two and three body nuclear collisions below 50 Mev is being developed. The procedure closely follows the channel packet method (CPM) used to compute scattering matrix elements for non-adiabatic molecular reactions.ootnotetextT.A.Niday and D.E.Weeks, Chem. Phys. Letters 308 (1999) 106 Currently, one degree of freedom calculations using a simple square well have been completed and a two body scattering calculation using the Yukawa potential is anticipated. To perform nuclear scattering calculations with the CPM that will incorporate the nucleon-nucleon tensor force, we plan to position initial reactant and product channel packets in the asymptotic limit on single coupled potential energy surfaces labeled by the spin, isospin, and total angular momentum of the reactant nucleons. The wave packets will propagated numerically using the split operator method augmented by a coordinate dependant unitary transformation used to diagonalize the potential. Scattering matrix elements will be determined by the Fourier transform of the correlation function between the evolving reactant and product wave packets. A brief outline of the Argonne v18 nucleon-nucleon potentialootnotetextR.B.Wiringa, V.G.J.Stoks, and R.Schiavilla, Physical Review C 51(1995) 38 and the proposed wave packet calculations will be presented.

  17. Network-timing-dependent plasticity.

    PubMed

    Delattre, Vincent; Keller, Daniel; Perich, Matthew; Markram, Henry; Muller, Eilif B

    2015-01-01

    Bursts of activity in networks of neurons are thought to convey salient information and drive synaptic plasticity. Here we report that network bursts also exert a profound effect on Spike-Timing-Dependent Plasticity (STDP). In acute slices of juvenile rat somatosensory cortex we paired a network burst, which alone induced long-term depression (LTD), with STDP-induced long-term potentiation (LTP) and LTD. We observed that STDP-induced LTP was either unaffected, blocked or flipped into LTD by the network burst, and that STDP-induced LTD was either saturated or flipped into LTP, depending on the relative timing of the network burst with respect to spike coincidences of the STDP event. We hypothesized that network bursts flip STDP-induced LTP to LTD by depleting resources needed for LTP and therefore developed a resource-dependent STDP learning rule. In a model neural network under the influence of the proposed resource-dependent STDP rule, we found that excitatory synaptic coupling was homeostatically regulated to produce power law distributed burst amplitudes reflecting self-organized criticality, a state that ensures optimal information coding.

  18. Network-timing-dependent plasticity

    PubMed Central

    Delattre, Vincent; Keller, Daniel; Perich, Matthew; Markram, Henry; Muller, Eilif B.

    2015-01-01

    Bursts of activity in networks of neurons are thought to convey salient information and drive synaptic plasticity. Here we report that network bursts also exert a profound effect on Spike-Timing-Dependent Plasticity (STDP). In acute slices of juvenile rat somatosensory cortex we paired a network burst, which alone induced long-term depression (LTD), with STDP-induced long-term potentiation (LTP) and LTD. We observed that STDP-induced LTP was either unaffected, blocked or flipped into LTD by the network burst, and that STDP-induced LTD was either saturated or flipped into LTP, depending on the relative timing of the network burst with respect to spike coincidences of the STDP event. We hypothesized that network bursts flip STDP-induced LTP to LTD by depleting resources needed for LTP and therefore developed a resource-dependent STDP learning rule. In a model neural network under the influence of the proposed resource-dependent STDP rule, we found that excitatory synaptic coupling was homeostatically regulated to produce power law distributed burst amplitudes reflecting self-organized criticality, a state that ensures optimal information coding. PMID:26106298

  19. Time dependence of PEB effects

    NASA Astrophysics Data System (ADS)

    Yanagishita, Yuichiro; Shigematsu, Kazumasa; Yanagida, Kimio

    1990-06-01

    Though simulations of PEB (Post Exposure Bake) on the basis of PAC diffusion mode! have been carried out by a number of researchers '' (2) , it has never been confirmed that those could predict experimental data caused by PEB' s effects accurately . Because no details of chemical reactions thernlly induced by PEB are known, fundamental parameters which determine PEB' s effects must be obtained experimentally. We have acquired the volume of changes of development rate function, RATE(M) by PEB with DRM monitoring for some types of photoresist . The values of diffusion length have been obtained by means of compareing experimental B (exposure ener) vs T (development time to clear) curves with simulated ones which is based on RATEOA) data. Their dependence on the baking time has been investigated with fixed FEB temperature and it has been proved that a progress of the diffusion saturates only in less than a few seconds when the diffusion length is about lO'-l5ncn, which is much shorter than the standing wave length(= 66nm, for G-line). Profiles of low contrast resist patterns can be improved by the decrease in development rate of slightly exposed areas by PEB. The effects on these resists depend on the baking time because the volume of the decrease grows with increasing FEB time. On the other hands, for high contrast resists PEB' s diffusion enhances their resolution while the decreases in development rate have little effect on them. Time dependence cannot be observed for these resists because the diffusion length remains constant with increasing FEB time.

  20. Electron-atomic-hydrogen ``elastic" scattering in the presence of a laser field

    NASA Astrophysics Data System (ADS)

    Li, S.-M.; Chen, J.; Zhou, Z.-F.

    2002-05-01

    Laser-assisted electron-atomic-hydrogen “elastic" scattering is studied in the first Born approximation. The initial and final states of projectile electron are described by the Volkov wavefunctions; the dressed state of target described by a time-dependent perturbative wavefunction in soft photon approximation. The laser modified cross-sections are calculated in two distinct geometries for laser polarization either parallel or perpendicular to the incident direction of electron. The numerical results shows that the multiphoton cross-sections oscillate by a few orders over the whole scattering angular region. The results for a parallel geometry oscillate more frequently in the intermediate angles; while the results for a perpendicular geometry oscillate more frequently in the forward and backward angles. At large scattering angles, the sum rule of Kroll and Watson is noticeably violated. The laser modification on summed total cross-section increases with field strength, but decreases with field frequency and polarization deviation from the incident direction.

  1. Time-dependent mean-field determination of the excitation energy in transfer reactions: Application to the reaction 238U on 12C at 6.14 MeV/nucleon

    NASA Astrophysics Data System (ADS)

    Scamps, G.; Rodríguez-Tajes, C.; Lacroix, D.; Farget, F.

    2017-02-01

    The internal excitation of nuclei after multinucleon transfer is estimated by using the time-dependent mean-field theory. Transfer probabilities for each channel as well as the energy loss after reseparation are calculated. By combining these two pieces of information, we show that the excitation energy distribution of the transfer fragments can be obtained separately for the different transfer channels. The method is applied to the reaction involving a 238U beam on a 12C target, which has recently been measured at GANIL. It is shown that the excitation energy calculated with the microscopic theory compares well with the experimental observation, provided that the competition with fusion is properly taken into account. The reliability of the excitation energy is further confirmed by the comparison with the phenomenological heavy-ion phase-space model at higher center-of-mass energies.

  2. Cyclotron resonance cooling by strong laser field

    SciTech Connect

    Tagcuhi, Toshihiro; Mima, Kunioka

    1995-12-31

    Reduction of energy spread of electron beam is very important to increase a total output radiation power in free electron lasers. Although several cooling systems of particle beams such as a stochastic cooling are successfully operated in the accelerator physics, these cooling mechanisms are very slow and they are only applicable to high energy charged particle beams of ring accelerators. We propose here a new concept of laser cooling system by means of cyclotron resonance. Electrons being in cyclotron motion under a strong magnetic field can resonate with circular polarized electromagnetic field, and the resonance take place selectively depending on the velocity of the electrons. If cyclotron frequency of electrons is equal to the frequency of the electromagnetic field, they absorb the electromagnetic field energy strongly, but the other electrons remain unchanged. The absorbed energy will be converted to transverse kinetic energy, and the energy will be dumped into the radiation energy through bremastrahlung. To build a cooling system, we must use two laser beams, where one of them is counter-propagating and the other is co-propagating with electron beam. When the frequency of the counter-propagating laser is tuned with the cyclotron frequency of fast electrons and the co-propagating laser is tuned with the cyclotron frequency of slow electrons, the energy of two groups will approach and the cooling will be achieved. We solve relativistic motions of electrons with relativistic radiation dumping force, and estimate the cooling rate of this mechanism. We will report optimum parameters for the electron beam cooling system for free electron lasers.

  3. Time-dependent diffusion in stellar atmospheres

    NASA Astrophysics Data System (ADS)

    Alecian, G.; Stift, M. J.; Dorfi, E. A.

    2011-12-01

    The chemical peculiarities of Ap stars are due to abundance stratifications produced by atomic diffusion in their outer layers. Theoretical models can predict such stratifications, but so far only provide equilibrium solutions which correspond to the maximum depth-dependent abundances for each element that can be supported by the radiation field. However, these stratifications are actually built up through a non-linear, time-dependent process which has never been modelled for realistic stellar atmospheres. Here, we present the first numerical simulations of time-dependent diffusion. We solve the continuity equation after having computed, as accurately as possible, atomic diffusion velocities (with and without a magnetic field) for a simplified fictitious - but still realistic - chemical element: cloudium. The direct comparison with existing observations is not the immediate aim of this work but rather a general understanding of how the stratification build-up proceeds in time and space. Our results raise serious questions as to the relevance of equilibrium solutions and reinforce the suspicion that certain accumulations of chemical elements might prove unstable.

  4. Ion and electron emission from silver nanoparticles in intense laser fields

    SciTech Connect

    Doeppner, T.; Fennel, Th.; Radcliffe, P.; Tiggesbaeumker, J.; Meiwes-Broer, K.-H.

    2006-03-15

    By a comparative analysis of the emission of highly charged ions and energetic electrons the interaction dynamics of intense femtosecond laser fields (10{sup 13}-10{sup 14} W/cm{sup 2}) with nanometer-sized silver clusters is investigated. Using dual laser pulses with variable optical delay the time-dependent cluster response is resolved. A dramatic increase both in the atomic charge state of the ions and the maximum electron kinetic energy is observed for a certain delay of the pulses. Corresponding Vlasov calculations on a metal cluster model system indicate that enhanced cluster ionization as well as the generation of fast electrons coincide with resonant plasmon excitation.

  5. Beyond carbon K-edge harmonic emission using a spatial and temporal synthesized laser field.

    PubMed

    Pérez-Hernández, J A; Ciappina, M F; Lewenstein, M; Roso, L; Zaïr, A

    2013-02-01

    We present numerical simulations of high-order harmonic generation in helium using a temporally synthesized and spatially nonhomogeneous strong laser field. The combination of temporal and spatial laser field synthesis results in a dramatic cutoff extension far beyond the usual semiclassical limit. Our predictions are based on the convergence of three complementary approaches: resolution of the three dimensional time dependent Schrödinger equation, time-frequency analysis of the resulting dipole moment, and classical trajectory extraction. A laser field synthesized both spatially and temporally has been proven capable of generating coherent extreme ultraviolet photons beyond the carbon K edge, an energy region of high interest as it can be used to initiate inner-shell dynamics and study time-resolved intramolecular attosecond spectroscopy.

  6. Nonsequential double ionization with time-dependent renormalized-natural-orbital theory

    NASA Astrophysics Data System (ADS)

    Brics, M.; Rapp, J.; Bauer, D.

    2014-11-01

    Recently introduced time-dependent renormalized-natural-orbital theory (TDRNOT) is tested on nonsequential double ionization (NSDI) of a numerically exactly solvable one-dimensional model He atom subject to few-cycle, 800-nm laser pulses. NSDI of atoms in strong laser fields is a prime example of nonperturbative, highly correlated electron dynamics. As such, NSDI is an important "worst-case" benchmark for any time-dependent few and many-body technique beyond linear response. It is found that TDRNOT reproduces the celebrated NSDI "knee," i.e., a many-order-of-magnitude enhancement of the double-ionization yield (as compared to purely sequential ionization) with only the ten most significant natural orbitals (NOs) per spin. Correlated photoelectron spectra—as "more differential" observables—require more NOs.

  7. Field mappers for laser material processing

    NASA Astrophysics Data System (ADS)

    Blair, Paul; Currie, Matthew; Trela, Natalia; Baker, Howard J.; Murphy, Eoin; Walker, Duncan; McBride, Roy

    2016-03-01

    The native shape of the single-mode laser beam used for high power material processing applications is circular with a Gaussian intensity profile. Manufacturers are now demanding the ability to transform the intensity profile and shape to be compatible with a new generation of advanced processing applications that require much higher precision and control. We describe the design, fabrication and application of a dual-optic, beam-shaping system for single-mode laser sources, that transforms a Gaussian laser beam by remapping - hence field mapping - the intensity profile to create a wide variety of spot shapes including discs, donuts, XY separable and rotationally symmetric. The pair of optics transform the intensity distribution and subsequently flatten the phase of the beam, with spot sizes and depth of focus close to that of a diffraction limited beam. The field mapping approach to beam-shaping is a refractive solution that does not add speckle to the beam, making it ideal for use with single mode laser sources, moving beyond the limits of conventional field mapping in terms of spot size and achievable shapes. We describe a manufacturing process for refractive optics in fused silica that uses a freeform direct-write process that is especially suited for the fabrication of this type of freeform optic. The beam-shaper described above was manufactured in conventional UV-fused silica using this process. The fabrication process generates a smooth surface (<1nm RMS), leading to laser damage thresholds of greater than 100J/cm2, which is well matched to high power laser sources. Experimental verification of the dual-optic filed mapper is presented.

  8. Laser plasma in a magnetic field

    SciTech Connect

    Kondo,K.; Kanesue, T.; Tamura, J.; Dabrowski, R.; Okamura, M.

    2009-09-20

    Laser Ion Source (LIS) is a candidate among various heavy ion sources. A high density plasma produced by Nd:YAG laser with drift velocity realizes high current and high charge state ion beams. In order to obtain higher charged particle ions, we had test experiments of LIS with a magnetic field by which a connement effect can make higher charged beams. We measured total current by Faraday Cup (FC) and analyzed charge distribution by Electrostatic Ion Analyzer (EIA). It is shown that the ion beam charge state is higher by a permanent magnet.

  9. Advances in time-dependent methods for multiphoton processes

    SciTech Connect

    Kulander, K.C.; Schafer, K.J.; Krause, J.L.

    1990-09-01

    This paper discusses recent theoretical results on above threshold ionization harmonic generation and high-frequency, high intensity suppression of ionization. These studies of multiphoton processes in atoms and molecules for short, intense pulsed optical lasers have been carried out using techniques which involve the explicit solution of the time-dependent Schroedinger equation. 43 refs., 5 figs.

  10. 21 CFR 886.1360 - Visual field laser instrument.

    Code of Federal Regulations, 2010 CFR

    2010-04-01

    ... 21 Food and Drugs 8 2010-04-01 2010-04-01 false Visual field laser instrument. 886.1360 Section... (CONTINUED) MEDICAL DEVICES OPHTHALMIC DEVICES Diagnostic Devices § 886.1360 Visual field laser instrument. (a) Identification. A visual field laser instrument is an AC-powered device intended to...

  11. 21 CFR 886.1360 - Visual field laser instrument.

    Code of Federal Regulations, 2013 CFR

    2013-04-01

    ... 21 Food and Drugs 8 2013-04-01 2013-04-01 false Visual field laser instrument. 886.1360 Section... (CONTINUED) MEDICAL DEVICES OPHTHALMIC DEVICES Diagnostic Devices § 886.1360 Visual field laser instrument. (a) Identification. A visual field laser instrument is an AC-powered device intended to...

  12. 21 CFR 886.1360 - Visual field laser instrument.

    Code of Federal Regulations, 2014 CFR

    2014-04-01

    ... 21 Food and Drugs 8 2014-04-01 2014-04-01 false Visual field laser instrument. 886.1360 Section... (CONTINUED) MEDICAL DEVICES OPHTHALMIC DEVICES Diagnostic Devices § 886.1360 Visual field laser instrument. (a) Identification. A visual field laser instrument is an AC-powered device intended to...

  13. 21 CFR 886.1360 - Visual field laser instrument.

    Code of Federal Regulations, 2011 CFR

    2011-04-01

    ... 21 Food and Drugs 8 2011-04-01 2011-04-01 false Visual field laser instrument. 886.1360 Section... (CONTINUED) MEDICAL DEVICES OPHTHALMIC DEVICES Diagnostic Devices § 886.1360 Visual field laser instrument. (a) Identification. A visual field laser instrument is an AC-powered device intended to...

  14. 21 CFR 886.1360 - Visual field laser instrument.

    Code of Federal Regulations, 2012 CFR

    2012-04-01

    ... 21 Food and Drugs 8 2012-04-01 2012-04-01 false Visual field laser instrument. 886.1360 Section... (CONTINUED) MEDICAL DEVICES OPHTHALMIC DEVICES Diagnostic Devices § 886.1360 Visual field laser instrument. (a) Identification. A visual field laser instrument is an AC-powered device intended to...

  15. Laser range pole field evaluation report

    NASA Technical Reports Server (NTRS)

    1973-01-01

    A field evaluation was made of the laser pole equipment. The basic plan for the evaluation was to expose the equipment to the actual people and environment for which it was intended and determine, through the use of the equipment, its resultant effectivity in terms of improved performance. Results show the equipment performed better than expected in the high elevation clean air of Colorado, and did as well in Tennessee.

  16. Time Dependent Fluid Occurrence Offshore Taiwan

    NASA Astrophysics Data System (ADS)

    Chen, L.

    2010-12-01

    Time Dependent Fluid Occurrence Offshore Taiwan Liwen Chenab, Wu-Cheng Chia, Char-Shine Liuc (mma@earth.sinica.edu.tw)(wchi@gate.sinica.edu.tw) ; aInstitute of Earth Sciences, Academia Sinica, Taipei, Taiwan bInstitute of Geosciences, National Taiwan University, Taipei, Taiwan ; cInstitute of Oceanography, National Taiwan University, Taipei, Taiwan Earthquake-induced groundwater flows have been observed recently. Such fluid flow might temporarily change the temperature field in the crust. Here we used seismically detected gas hydrate under seafloor to study the temperature fields at a few hundred meters subbottom depth before, and after the 2006 Henchuan earthquake (Mw7.0). We used the hydrate-related bottom-simulating-reflector (BSR) in seismic profiles to study the effects of gas/fluid migration on the BSR attributes. We have conducted two seismic experiments before and after the earthquake across the same transects near the hypocenter of the earthquake using similar air gun arrays and streamers. By analyzing this unique dataset, we found enhanced BSR reflectivity in average after the earthquake (~0.03), but the Sea-floor reflectivity is very similar (~0.5). We also found changed amplitudes versus offset (AVO) in the dataset (the gradient of reflection coefficient versus the angles was ~-0.34). We interpret these results as a consequence of earthquake-induced gas and fluid migration, bringing the gases underneath the BSR, thus the enhanced reflection coefficients. Next we will explore new methods to use the BSR as a flow meter. Using time-dependent seismic attribute analyses across transects before and after a large earthquake, we found strong evidences of earthquake-related fluid migrations and possibly associated temperature perturbations. This is among the first studies to document such feature in the offshore region.

  17. Characterization of the time-dependent strain field at seismogenic depths using first-motion focal mechanisms: Observations of large-scale decadal variations in stress along the San Andrea fault system

    USGS Publications Warehouse

    Sipkin, S.A.; Silver, P.G.

    2003-01-01

    We present a method for summing moment tensors derived from first-motion focal mechanisms to study temporal dependence in features of the subsurface regional strain field. Time-dependent processes are inferred by comparing mechanisms summed over differing time periods. We apply this methodology to seismogenic zones in central and southern California using focal mechanisms produced by the Northern and Southern California Seismograph Networks for events during 1980-1999. We find a consistent pattern in both the style of deformation (strike-slip versus compressional) and seismicity rate across the entire region. If these temporal variations are causally related, it suggests a temporal change in the regional-scale stress field. One change consistent with the observations is a rotation in the regional maximum horizontal compressive stress direction, followed by a reversal to the original direction. Depending upon the dominant style of deformation locally, this change in orientation of the regional stress will tend to either enhance or hinder deformation. The mode of enhanced deformation can range from increased microseismicity and creep to major earthquakes. We hypothesize that these temporal changes in the regional stress field are the result of subtle changes in apparent relative plate motion between the Pacific and North American plates, perhaps due to long-range postseismic stress diffusion. Others have hypothesized that small changes in plate motion over thousands of years, and/or over decades, are responsible for changes in the style of deformation in southern California. We propose that such changes, over the course of just a few years, also affect the style of deformation.

  18. Photoassociation dynamics driven by a modulated two-color laser field

    SciTech Connect

    Zhang Wei; Zhao Zeyu; Xie Ting; Wang Gaoren; Huang Yin; Cong Shulin

    2011-11-15

    Photoassociation (PA) dynamics of ultracold cesium atoms steered by a modulated two-color laser field E(t)=E{sub 0}f(t)cos((2{pi}/T{sub p})-{phi})cos({omega}{sub L}t) is investigated theoretically by numerically solving the time-dependent Schroedinger equation. The PA dynamics is sensitive to the phase of envelope (POE) {phi} and the period of the envelope T{sub p}, which indicates that it can be controlled by varying POE {phi} and period T{sub p}. Moreover, we introduce the time- and frequency-resolved spectrum to illustrate how the POE {phi} and the period T{sub p} influence the intensity distribution of the modulated laser pulse and hence change the time-dependent population distribution of photoassociated molecules. When the Gaussian envelope contains a few oscillations, the PA efficiency is also dependent on POE {phi}. The modulated two-color laser field is available in the current experiment based on laser mode-lock technology.

  19. Probing Time-Dependent Molecular Dipoles on the Attosecond Time Scale

    NASA Astrophysics Data System (ADS)

    Neidel, Ch.; Klei, J.; Yang, C.-H.; Rouzée, A.; Vrakking, M. J. J.; Klünder, K.; Miranda, M.; Arnold, C. L.; Fordell, T.; L'Huillier, A.; Gisselbrecht, M.; Johnsson, P.; Dinh, M. P.; Suraud, E.; Reinhard, P.-G.; Despré, V.; Marques, M. A. L.; Lépine, F.

    2013-07-01

    Photoinduced molecular processes start with the interaction of the instantaneous electric field of the incident light with the electronic degrees of freedom. This early attosecond electronic motion impacts the fate of the photoinduced reactions. We report the first observation of attosecond time scale electron dynamics in a series of small- and medium-sized neutral molecules (N2, CO2, and C2H4), monitoring time-dependent variations of the parent molecular ion yield in the ionization by an attosecond pulse, and thereby probing the time-dependent dipole induced by a moderately strong near-infrared laser field. This approach can be generalized to other molecular species and may be regarded as a first example of molecular attosecond Stark spectroscopy.

  20. Prediction of I2P 1/2-->2P 3/2 transition lineshapes from 3-D, time dependent simulations of chemical oxygen-iodine laser (COIL) flowfields

    NASA Astrophysics Data System (ADS)

    Madden, Timothy J.

    2008-02-01

    The lineshape of the I2P 1/2-->2P 3/2 transition provides a means to ascertain a variety of useful information regarding the performance of the chemical oxygen-iodine laser (COIL). The value at the center of the lineshape, commonly referred to as the 'line center,' is proportional to the laser amplification on the I2P 1/2-->2P 3/2 transition. The infinite integral of the lineshape is proportional to the number density of the ground and excited states of atomic iodine in the gas, indicating the degree of I II dissociation. And the width of the lineshape indicates the amount of broadening of the transition, both due to collisional and Doppler shift effects. As the Doppler shift is proportional to velocity, the width of the transition can be used to estimate the degree of random molecular motion in the gas, expressed in macroscopic terms as temperature. A Doppler shift to the frequencies in the transition can also occur through the straight-line, bulk motion of the gas, and this can be used to examine the velocity field of the gas. However, the flow may experience rotation through the presence of eddies carried within the gas, and these too may contribute to the Doppler shift of the lineshape frequencies. Given that eddies by virtue of their positive and negative velocity components can induce positive and negative Doppler shift, the widening of the lineshape is similar to thermal motion which also includes positive and negative velocities. Thus, when interpreting transition lineshapes, if some account is not made for both thermal and rotational motion, the effect of either physical process will be over-estimated. The work discussed here is oriented toward examining the interplay between the gas dynamics and the lineshape of the I2P 1/2-->2P 3/2 transition, and in turn determine the ramifications for the use of spectroscopic lineshape based diagnostics and interpretation of their data. These efforts in turn are directly linked to efforts improve the understanding of

  1. Momentum space iterative solution of the time-dependent Schrödinger equation

    SciTech Connect

    Kiss, G. Zs.; Borbély, S.; Nagy, L.

    2013-11-13

    We present a novel approach, the iterative solution of the time-dependent Schrödinger equation (iTDSE model), for the investigation of atomic systems interacting with external laser fields. This model is the extension of the momentum-space strong-field approximation (MSSFA) [1], in which the Coulomb potential was considered only as a first order perturbation. In the iTDSE approach higher order terms were gradually introduced until convergence was achieved. Benchmark calculations were done on the hydrogen atom, and the obtained results were compared to the direct numerical solution [2].

  2. Spectral methods for time dependent problems

    NASA Technical Reports Server (NTRS)

    Tadmor, Eitan

    1990-01-01

    Spectral approximations are reviewed for time dependent problems. Some basic ingredients from the spectral Fourier and Chebyshev approximations theory are discussed. A brief survey was made of hyperbolic and parabolic time dependent problems which are dealt with by both the energy method and the related Fourier analysis. The ideas presented above are combined in the study of accuracy stability and convergence of the spectral Fourier approximation to time dependent problems.

  3. Infrared Blobs : Time-dependent Flags

    NASA Astrophysics Data System (ADS)

    McCullough, P. R.; Mack, J.; Dulude, M.; Hilbert, B.

    2014-10-01

    We describe the creation of time-dependent flags for pixels associated with "blobs" on the WFC3 IR detector. We detect the blobs on flat fields obtained by repeated observations of the night side of the Earth. We provide the most complete census of IR blobs' positions, radii, and times of first appearance. In aggregate, a set of 46 blobs, 27 "strong" and 19 "medium" in their effective scattering cross section, affect slightly less than 1% of the pixels of the detector. A second set of 81 "weak" (and typically smaller) blobs affect another 1% of the pixels. In the past, the "blob" flag, bit 9 (i.e. value = 512) in the data quality (DQ) array described in Table 2.5 of the WFC3 Data Handbook (Rajan et al. 2010) has been a static 2-D array; henceforth a set of such arrays, each associated with a "use after" date corresponding to the appearance of one or more new blobs, can be used. We prepared such DQ arrays using the 46 "strong" and "medium" blobs and discuss why we did not include the fainter blobs therein. As an added data product, we create and test a blob flat field that corrects the effects of blobs on extended emission; however, it should not be applied if stellar photometry is the goal.

  4. Time-dependent density functional theory/discrete reaction field spectra of open shell systems: The visual spectrum of [FeIII(PyPepS)2]- in aqueous solution.

    PubMed

    van Duijnen, Piet Th; Greene, Shannon N; Richards, Nigel G J

    2007-07-28

    We report the calculated visible spectrum of [FeIII(PyPepS)2]- in aqueous solution. From all-classical molecular dynamics simulations on the solute and 200 water molecules with a polarizable force field, 25 solute/solvent configurations were chosen at random from a 50 ps production run and subjected the systems to calculations using time-dependent density functional theory (TD-DFT) for the solute, combined with a solvation model in which the water molecules carry charges and polarizabilities. In each calculation the first 60 excited states were collected in order to span the experimental spectrum. Since the solute has a doublet ground state several excitations to states are of type "three electrons in three orbitals," each of which gives rise to a manifold of a quartet and two doublet states which cannot properly be represented by single Slater determinants. We applied a tentative scheme to analyze this type of spin contamination in terms of Delta and Delta transitions between the same orbital pairs. Assuming the associated states as pure single determinants obtained from restricted calculations, we construct conformation state functions (CFSs), i.e., eigenfunctions of the Hamiltonian Sz and S2, for the two doublets and the quartet for each Delta,Delta pair, the necessary parameters coming from regular and spin-flip calculations. It appears that the lower final states remain where they were originally calculated, while the higher states move up by some tenths of an eV. In this case filtering out these higher states gives a spectrum that compares very well with experiment, but nevertheless we suggest investigating a possible (re)formulation of TD-DFT in terms of CFSs rather than determinants.

  5. On refractive processes in strong laser field quantum electrodynamics

    SciTech Connect

    Di Piazza, A.

    2013-11-15

    Refractive processes in strong-field QED are pure quantum processes, which involve only external photons and the background electromagnetic field. We show analytically that such processes occurring in a plane-wave field and involving external real photons are all characterized by a surprisingly modest net exchange of energy and momentum with the laser field, corresponding to a few laser photons, even in the limit of ultra-relativistic laser intensities. We obtain this result by a direct calculation of the transition matrix element of an arbitrary refractive QED process and accounting exactly for the background plane-wave field. A simple physical explanation of this modest net exchange of laser photons is provided, based on the fact that the laser field couples with the external photons only indirectly through virtual electron–positron pairs. For stronger and stronger laser fields, the pairs cover a shorter and shorter distance before they annihilate again, such that the laser can transfer to them an energy corresponding to only a few photons. These results can be relevant for the future experiments aiming to test strong-field QED at present and next-generation facilities. -- Highlights: •Investigation of the one-loop amplitude of refractive QED processes in a laser field. •The amplitude is suppressed for a large number of net-exchanged laser photons. •Suggestion for first observation of high-nonlinear vacuum effects in a laser field.

  6. Fragmentation dynamics of Ar2^+ dimers in intense laser fields

    NASA Astrophysics Data System (ADS)

    Magrakvelidze, M.; Wu, J.; Dörner, R.; Thumm, U.

    2012-06-01

    We studied the fragmentation dynamics of the Ar2 dimers in 790 nm pump and 1400 nm probe pulses with intensities of 10^14 W/cm^2 by analyzing kinetic energy release (KER) spectra as a function of the pump probe delay. The KER spectra are measured by detecting Ar-ion fragments in a COLTRIMS [1] setup and are compared with model calculations based on the numerical propagations of the time-dependent Schr"odinger equation [2]. The measured spectra are best reproduced by two-state calculations that include the adiabatic electronic states I(1/2)u and II(1/2)g of Ar2^+, dipole coupled in the pump- and probe-laser electric fields. [4pt] [1] J. Wu, A. Vredenborg, B. Ulrich, L. Ph. H. Schmidt, M. Meckel, S. Voss, H. Sann, H. Kim, T. Jahnke, and R. D"orner, PRA 83, 061403(R) (2011) [0pt] [2] M. Magrakvelidze, F. He, Th. Niederhausen, I. V. Litvinyuk, and U. Thumm, PRA 79, 033410 (2009).

  7. Ultrafast Modulation of Semiconductor Lasers Through a Terahertz Field

    NASA Technical Reports Server (NTRS)

    Ning, Cun-Zheng; Hughes, Steven; Citrin, David

    1998-01-01

    We demonstrate, by means of numerical simulation, a new mechanism to modulate and switch semiconductor lasers at THz and sub-THz frequency rates. A sinusoidal terahertz field applied to a semiconductor laser heats the electron-hole plasma and consequently modifies the optical susceptibility. This allows an almost linear modulation of the output power of tile semiconductor laser and leads to a faithful reproduction of the terahertz-field waveform in the emitted laser intensity.

  8. Laser-sub-cycle two-dimensional electron-momentum mapping using orthogonal two-color fields

    NASA Astrophysics Data System (ADS)

    Zhang, Li; Xie, Xinhua; Roither, Stefan; Kartashov, Daniil; Wang, YanLan; Wang, ChuanLiang; Schöffler, Markus; Shafir, Dror; Corkum, Paul B.; Baltuška, Andrius; Ivanov, Igor; Kheifets, Anatoli; Liu, XiaoJun; Staudte, André; Kitzler, Markus

    2014-12-01

    We study laser-sub-cycle control over electron trajectories concomitantly in space and time using orthogonally polarized two-color laser fields. We compare experimental photoelectron spectra of neon recorded by coincidence momentum imaging with photoelectron spectra obtained by semiclassical and numerical solutions of the time-dependent Schrödinger equation. We find that a resolution of a quarter optical cycle in the photoelectron trajectories can be achieved. It is shown that depending on their sub-cycle birth time the trajectories of photoelectrons are affected differently by the ion's Coulomb field.

  9. Time-dependent density-functional description of nuclear dynamics

    NASA Astrophysics Data System (ADS)

    Nakatsukasa, Takashi; Matsuyanagi, Kenichi; Matsuo, Masayuki; Yabana, Kazuhiro

    2016-10-01

    The basic concepts and recent developments in the time-dependent density-functional theory (TDDFT) for describing nuclear dynamics at low energy are presented. The symmetry breaking is inherent in nuclear energy density functionals, which provides a practical description of important correlations at the ground state. Properties of elementary modes of excitation are strongly influenced by the symmetry breaking and can be studied with TDDFT. In particular, a number of recent developments in the linear response calculation have demonstrated their usefulness in the description of collective modes of excitation in nuclei. Unrestricted real-time calculations have also become available in recent years, with new developments for quantitative description of nuclear collision phenomena. There are, however, limitations in the real-time approach; for instance, it cannot describe the many-body quantum tunneling. Thus, the quantum fluctuations associated with slow collective motions are explicitly treated assuming that time evolution of densities is determined by a few collective coordinates and momenta. The concept of collective submanifold is introduced in the phase space associated with the TDDFT and used to quantize the collective dynamics. Selected applications are presented to demonstrate the usefulness and quality of the new approaches. Finally, conceptual differences between nuclear and electronic TDDFT are discussed, with some recent applications to studies of electron dynamics in the linear response and under a strong laser field.

  10. Stability on Time-Dependent Domains

    NASA Astrophysics Data System (ADS)

    Knobloch, E.; Krechetnikov, R.

    2014-06-01

    We explore the key differences in the stability picture between extended systems on time-fixed and time-dependent spatial domains. As a paradigm, we take the complex Swift-Hohenberg equation, which is the simplest nonlinear model with a finite critical wavenumber, and use it to study dynamic pattern formation and evolution on time-dependent spatial domains in translationally invariant systems, i.e., when dilution effects are absent. In particular, we discuss the effects of a time-dependent domain on the stability of spatially homogeneous and spatially periodic base states, and explore its effects on the Eckhaus instability of periodic states. New equations describing the nonlinear evolution of the pattern wavenumber on time-dependent domains are derived, and the results compared with those on fixed domains. Pattern coarsening on time-dependent domains is contrasted with that on fixed domains with the help of the Cahn-Hilliard equation extended here to time-dependent domains. Parallel results for the evolution of the Benjamin-Feir instability on time-dependent domains are also given.

  11. Time-dependent photoelectron angular distributions

    NASA Astrophysics Data System (ADS)

    Wang, Xiangyang

    1999-09-01

    I show that the angular distribution of electrons photoionized from gas phase targets by short light pulses is time-dependent, when the orbital momentum composition of the photocurrent changes with excitation energy so evolves with the time of detection. A theory of time- dependent photoionization is outlined and general formulas of time-dependent photoelectron flux and angular distribution are given. Two general propagator methods suitable to describe the time-dependent photoionization and scattering processes are developed. The photoionization process is viewed as a local excitation followed by a half scattering. The local excitation process is solved theoretically in a small region around the target core. This approach has been generalized to describe the evolution of a wavepacket in an unbound system. An asymptotic propagator theorem is discovered and used to derive analytic expressions for asymptotic propagators. The origin of the time dependence is explored by parameterizing the time delay and orbital momentum coupling in a two channel model. K-shell photoionization of N2 and CO are calculated with this time- dependent photoionization theory, implemented using a multiple scattering model. Numerical results demonstrate that the time dependence of photoelectron angular distributions is a realistic effect.

  12. Atomic phenomena in bichromatic laser fields

    NASA Astrophysics Data System (ADS)

    Ehlotzky, Fritz

    2001-05-01

    We present a review of work that has been done during the last 10 years on atomic scattering and reaction processes in bichromatic laser fields. Of particular interest will be the case where the field is composed of two components of commensurate frequencies, usually consisting of a fundamental component ω and one of its low harmonics 2 ω or 3 ω. These two components are in general out of phase by an angle ϕ. The above processes are then investigated as a function of the relative phase ϕ. This procedure was termed the coherent phase control (CPC) of the atomic process considered. The idea was originally born in molecular physics as a possible means to manipulate molecular reactions.

  13. Nuclear classical dynamics of H2 in an intense laser field

    NASA Astrophysics Data System (ADS)

    Sami, Firoozeh; Vafaee, Mohsen; Shokri, Babak

    2011-08-01

    In the first part of this paper, the different distinguishable pathways and regions of the single and sequential double ionization are determined and discussed. It is shown that there are two distinguishable pathways for the single ionization and four distinct pathways for the sequential double ionization. It is also shown that there are two and three different regions of space which are related to the single and double ionization, respectively. In the second part of the paper, the time-dependent Schrödinger and Newton equations are solved simultaneously for the electrons and the nuclei of H2, respectively. The electron and nuclei dynamics are separated on the basis of the adiabatic approximation. The soft-core potential is used to model the electrostatic interaction between the electrons and the nuclei. A variety of wavelengths (390, 532 and 780 nm) and intensities (5 × 1014 and 5 × 1015 W cm-2) of the ultrashort intense laser pulses with a sinus second-order envelope function are used. The behaviour of the time-dependent classical nuclear dynamics in the absence and presence of the laser field is investigated and compared. In the absence of the laser field, there are three distinct sections for the nuclear dynamics on the electronic ground state energy curve. The bond hardening phenomenon does not appear in this classical nuclear dynamics simulation.

  14. High-harmonic spectra from time-dependent two-particle reduced-density-matrix theory

    NASA Astrophysics Data System (ADS)

    Lackner, Fabian; Březinová, Iva; Sato, Takeshi; Ishikawa, Kenichi L.; Burgdörfer, Joachim

    2017-03-01

    The ab initio description of the nonlinear response of many-electron systems to strong-laser fields remains a major challenge. In order to address larger systems, alternative methods need to be developed that bypass the exponential scaling with particle number inherent to conventional wave-function-based approaches. In this paper we present a fully three-dimensional implementation of the time-dependent two-particle reduced-density-matrix (TD-2RDM) method for many-electron atoms. We benchmark this approach by a comparison with multiconfigurational time-dependent Hartree-Fock results for the harmonic spectra of beryllium and neon. We show that the TD-2RDM is very well suited to describe the nonlinear atomic response and to reveal the influence of electron-correlation effects.

  15. Time dependent friction in a free gas

    NASA Astrophysics Data System (ADS)

    Fanelli, Cristiano; Sisti, Francesco; Stagno, Gabriele V.

    2016-03-01

    We consider a body moving in a perfect gas, described by the mean-field approximation and interacting elastically with the body, we study the friction exerted by the gas on the body fixed at constant velocities. The time evolution of the body in this setting was studied in Caprino et al. [Math. Phys. 264, 167-189 (2006)], Caprino et al. [Math. Models Methods Appl. Sci. 17, 1369-1403 (2007)], and Cavallaro [Rend. Mat. Appl. 27, 123-145 (2007)] for object with simple shape; the first study where a simple kind of concavity was considered was in Sisti and Ricciuti [SIAM J. Math. Anal. 46, 3759-3611 (2014)], showing new features in the dynamic but not in the friction term. The case of more general shape of the body was left out for further difficulties, and we believe indeed that there are actually non-trivial issues to be faced for these more general cases. To show this and in the spirit of getting a more realistic perspective in the study of friction problems, in this paper, we focused our attention on the friction term itself, studying its behavior on a body with a more general kind of concavity and fixed at constant velocities. We derive the expression of the friction term for constant velocities, we show how it is time dependent, and we give its exact estimate in time. Finally, we use this result to show the absence of a constant velocity in the actual dynamic of such a body.

  16. High-order-harmonic generation from Rydberg atoms driven by plasmon-enhanced laser fields

    NASA Astrophysics Data System (ADS)

    Tikman, Y.; Yavuz, I.; Ciappina, M. F.; Chacón, A.; Altun, Z.; Lewenstein, M.

    2016-02-01

    We theoretically investigate high-order-harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should exceed a certain threshold in order to stimulate HHG when noble gas atoms in their ground state are used as an active medium. One way to enhance the coherent light coming from a conventional laser oscillator is to take advantage of the amplification obtained by the so-called surface plasmon polaritons, created when a low-intensity laser field is focused onto a metallic nanostructure. The main limitation of this scheme is the low damage threshold of the materials employed in the nanostructure engineering. In this work we propose the use of Rydberg atoms, driven by spatially inhomogeneous, plasmon-enhanced laser fields, for HHG. We exhaustively discuss the behavior and efficiency of these systems in the generation of coherent harmonic emission. Toward this aim we numerically solve the time-dependent Schrödinger equation for an atom, with an electron initially in a highly excited n th Rydberg state, located in the vicinity of a metallic nanostructure. In this zone the electric field changes spatially on scales relevant for the dynamics of the laser-ionized electron. We first use a one-dimensional model to investigate systematically the phenomena. We then employ a more realistic situation, in which the interaction of a plasmon-enhanced laser field with a three-dimensional hydrogen atom is modeled. We discuss the scaling of the relevant input parameters with the principal quantum number n of the Rydberg state in question and demonstrate that harmonic emission can be achieved from Rydberg atoms well below the damage threshold, thus without deterioration of the geometry and properties of the metallic nanostructure.

  17. Formation of the domain structure in CLN under the pyroelectric field induced by pulse infrared laser heating

    SciTech Connect

    Shur, V. Ya.; Kosobokov, M. S.; Mingaliev, E. A.; Karpov, V. R.

    2015-10-15

    The evolution of the self-assembled quasi-regular micro- and nanodomain structures after pulse infrared laser irradiation in congruent lithium niobate crystal was studied by in situ optical observation. Several scenarios of domain kinetics represented covering of the irradiated zone by nets of the separated domain chains and rays have been revealed. The time dependence of the total domain length was analyzed in terms of modified Kolmogorov-Avrami theory. The domain structure evolution was attributed to the action of pyroelectric field appeared during cooling. The time dependence of the spatial distribution of the pyroelectric field during pulse laser heating and subsequent cooling was calculated by finite element method. The results of computer simulation allowed us to explain the experimental results and can be used for creation of tailored domain structures thus opening the new abilities of the submicron-scale domain engineering in ferroelectrics.

  18. Fast electrons from electron-ion collisions in strong laser fields

    NASA Astrophysics Data System (ADS)

    Kull, H.-J.; Tikhonchuk, V. T.

    2005-06-01

    Electron-ion collisions in the presence of a strong laser field lead to a distribution of fast electrons with maximum energy Emax=(k0+2v0)2/2(a.u.), where k0 is the impact and v0 the quiver velocity of the electron. The energy spectrum is calculated by two approaches: (1) The time-dependent Schrödinger equation is numerically solved for wave packet scattering from a one-dimensional softcore Coulomb potential. Multiphoton energy spectra are obtained demonstrating a separation of the energy spectrum into an exponential distribution for transmission and a plateau distribution for reflection. (2) The energy spectrum is analytically calculated in the framework of classical instantaneous Coulomb collisions with random impact parameters and random phases of the laser field. An exact solution for the energy spectrum is obtained from which the fraction of fast electrons in the plateau region can be estimated.

  19. Hole dynamics and spin currents after ionization in strong circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Barth, Ingo; Smirnova, Olga

    2014-10-01

    We apply the time-dependent analytical R-matrix theory to develop a movie of hole motion in a Kr atom upon ionization by strong circularly polarized field. We find rich hole dynamics, ranging from rotation to swinging motion. The motion of the hole depends on the final energy and the spin of the photoelectron and can be controlled by the laser frequency and intensity. Crucially, hole rotation is a purely non-adiabatic effect, completely missing in the framework of quasistatic (adiabatic) tunneling theories. We explore the possibility to use hole rotation as a clock for measuring ionization time. Analyzing the relationship between the relative phases in different ionization channels we show that in the case of short-range electron-core interaction the hole is always initially aligned along the instantaneous direction of the laser field, signifying zero delays in ionization. Finally, we show that strong-field ionization in circular fields creates spin currents (i.e. different flow of spin-up and spin-down density in space) in the ions. This phenomenon is intimately related to the production of spin-polarized electrons in strong laser fields Barth and Smirnova (2013 Phys. Rev. A 88 013401). We demonstrate that rich spin dynamics of electrons and holes produced during strong field ionization can occur in typical experimental conditions and does not require relativistic intensities or strong magnetic fields.

  20. Topic 5: Time-Dependent Behavior

    SciTech Connect

    Pfeiffer, P.A.; Tanabe, Tada-aki

    1991-12-31

    This chapter is a report of the material presented at the International Workshop on Finite Element Analysis of Reinforced Concrete, Session 4 -- Time Dependent Behavior, held at Columbia University, New York on June 3--6, 1991. Dr. P.A. Pfeiffer presented recent developments in time-dependent behavior of concrete and Professor T. Tanabe presented a review of research in Japan on time-dependent behavior of concrete. The chapter discusses the recent research of time-dependent behavior of concrete in the past few years in both the USA-European and Japanese communities. The author appreciates the valuable information provided by Zdenek P. Bazant in preparing the USA-European Research section.

  1. Nature of the strong field capabilities of lasers

    NASA Astrophysics Data System (ADS)

    Reiss, H. R.

    2013-05-01

    Research with lasers of extremely high intensity has been proposed in terms of tunneling and the "Schwinger Limit", which refers to breakdown of the vacuum into electron-positron pairs caused by a static or quasistatic electric field. The difficulty is that lasers produce transverse fields, wherein the electric and magnetic fields form a mutually orthogonal triad with the direction of propagation. Tunneling, including the Schwinger Limit, relates to longitudinal fields, in which the direction of the electric field vector is the only preferred direction. Transverse fields propagate indefinitely without inputs from source or current distributions. By contrast, longitudinal fields require continuing contributions from external source or current distributions. Failure to distinguish between longitudinal and transverse fields is consequential in that some proposed applications of very high intensity lasers pertain only to tunneling processes, but not to laser fields. A related difficulty is the flawed notion that tunneling constitutes a low-frequency limit of laser-induced processes. A counter-indication is that the ponderomotive potential of a charged particle in a laser field is proportional to the inverse square of the field frequency. Thus there is no possible approach to a zero-frequency laser field. The Göppert-Mayer gauge transformation of atomic physics makes possible a limited correspondence between transverse and longitudinal fields. The correspondence fails at both high and, most importantly, at low field frequencies. Vacuum pair production does not require the Schwinger Limit, but can be achieved at much lower intensities.

  2. Invariants for time-dependent Hamiltonian systems.

    PubMed

    Struckmeier, J; Riedel, C

    2001-08-01

    An exact invariant is derived for n-degree-of-freedom Hamiltonian systems with general time-dependent potentials. The invariant is worked out in two equivalent ways. In the first approach, we define a special Ansatz for the invariant and determine its time-dependent coefficients. In the second approach, we perform a two-step canonical transformation of the initially time-dependent Hamiltonian to a time-independent one. The invariant is found to contain a function of time f(2)(t), defined as a solution of a linear third-order differential equation whose coefficients depend in general on the explicitly known configuration space trajectory that follows from the system's time evolution. It is shown that the invariant can be interpreted as the time integral of an energy balance equation. Our result is applied to a one-dimensional, time-dependent, damped non-linear oscillator, and to a three-dimensional system of Coulomb-interacting particles that are confined in a time-dependent quadratic external potential. We finally show that our results can be used to assess the accuracy of numerical simulations of time-dependent Hamiltonian systems.

  3. Atoms and molecules in intense laser fields: gauge invariance of theory and models

    NASA Astrophysics Data System (ADS)

    Bandrauk, A. D.; Fillion-Gourdeau, F.; Lorin, E.

    2013-08-01

    Gauge invariance was discovered in the development of classical electromagnetism and was required when the latter was formulated in terms of the scalar and vector potentials. It is now considered to be a fundamental principle of nature, stating that different forms of these potentials yield the same physical description: they describe the same electromagnetic field as long as they are related to each other by gauge transformations. Gauge invariance can also be included into the quantum description of matter interacting with an electromagnetic field by assuming that the wavefunction transforms under a given local unitary transformation. The result of this procedure is a quantum theory describing the coupling of electrons, nuclei and photons. Therefore, it is a very important concept: it is used in almost every field of physics and it has been generalized to describe electroweak and strong interactions in the standard model of particles. A review of quantum mechanical gauge invariance and general unitary transformations is presented for atoms and molecules in interaction with intense short laser pulses, spanning the perturbative to highly nonlinear non-perturbative interaction regimes. Various unitary transformations for a single spinless particle time-dependent Schrödinger equation (TDSE) are shown to correspond to different time-dependent Hamiltonians and wavefunctions. Accuracy of approximation methods involved in solutions of TDSEs such as perturbation theory and popular numerical methods depend on gauge or representation choices which can be more convenient due to faster convergence criteria. We focus on three main representations: length and velocity gauges, in addition to the acceleration form which is not a gauge, to describe perturbative and non-perturbative radiative interactions. Numerical schemes for solving TDSEs in different representations are also discussed. A final brief discussion of these issues for the relativistic time-dependent Dirac equation

  4. Radiation-reaction trapping of electrons in extreme laser fields.

    PubMed

    Ji, L L; Pukhov, A; Kostyukov, I Yu; Shen, B F; Akli, K

    2014-04-11

    A radiation-reaction trapping (RRT) of electrons is revealed in the near-QED regime of laser-plasma interaction. Electrons quivering in laser pulse experience radiation reaction (RR) recoil force by radiating photons. When the laser field reaches the threshold, the RR force becomes significant enough to compensate for the expelling laser ponderomotive force. Then electrons are trapped inside the laser pulse instead of being scattered off transversely and form a dense plasma bunch. The mechanism is demonstrated both by full three-dimensional particle-in-cell simulations using the QED photonic approach and numerical test-particle modeling based on the classical Landau-Lifshitz formula of RR force. Furthermore, the proposed analysis shows that the threshold of laser field amplitude for RRT is approximately the cubic root of laser wavelength over classical electron radius. Because of the pinching effect of the trapped electron bunch, the required laser intensity for RRT can be further reduced.

  5. Pedagogical Aspects of Time-Dependent Rotation Operators.

    ERIC Educational Resources Information Center

    Leubner, C.

    1980-01-01

    Describes the reformulation of a classical magnetic moment interacting with various magnetic field configurations in terms of coordinate-free, time-dependent rotation operators. This approach provides useful exercises for the manipulation of three-dimensional rotation operators and provides examples for a number of quantum-mechanics related…

  6. Strong-field atomic ionization in an elliptically polarized laser field and a constant magnetic field

    NASA Astrophysics Data System (ADS)

    Rylyuk, V. M.

    2016-05-01

    Within the framework of the quasistationary quasienergy state (QQES) formalism, the tunneling and multiphoton ionization of atoms and ions subjected to a perturbation by a high intense laser radiation field of an arbitrary polarization and a constant magnetic field are considered. On the basis of the exact solution of the Schrödinger equation and the Green's function for the electron moving in an arbitrary laser field and crossed constant electric and magnetic fields, the integral equation for the complex quasienergy and the energy spectrum of the ejected electron are derived. Using the "imaginary-time" method, the extremal subbarrier trajectory of the photoelectron moving in a nonstationary laser field and a constant magnetic field are considered. Within the framework of the QQES formalism and the quasiclassical perturbation theory, ionization rates when the Coulomb interaction of the photoelectron with the parent ion is taken into account at arbitrary values of the Keldysh parameter are derived. The high accuracy of rates is confirmed by comparison with the results of numerical calculations. Simple analytical expressions for the ionization rate with the Coulomb correction in the tunneling and multiphoton regimes in the case of an elliptically polarized laser beam propagating at an arbitrary angle to the constant magnetic field are derived and discussed. The limits of small and large magnetic fields and low and high frequency of a laser field are considered in details. It is shown that in the presence of a nonstationary laser field perturbation, the constant magnetic field may either decrease or increase the ionization rate. The analytical consideration and numerical calculations also showed that the difference between the ionization rates for an s electron in the case of right- and left-elliptically polarized laser fields is especially significant in the multiphoton regime for not-too-high magnetic fields and decreases as the magnetic field increases. The paper

  7. Time-dependent Flare Models with MALI

    NASA Astrophysics Data System (ADS)

    Kašparová, J.; Heinzel, P.; Varady, M.; Karlický, M.

    2003-01-01

    Temporal variations of Hα line profile intensities related to electron beams are presented. We show first results of time dependent simulations of a chromospheric response to a 1 sec monoenergetic electron beam. 1-D hydrodynamic code together with particle representation of the beam have been used to calculate atmospheric evolution. Time dependent radiative transfer problem has been solved for the resulting atmosphere in the MALI approach, using the Crank-Nicholson implicit scheme. Non-thermal collisional rates were included in linearised equations of statistical equilibrium.

  8. Angle-Dependent Ionization of Small Molecules by Time-Dependent Configuration Interaction and an Absorbing Potential.

    PubMed

    Krause, Pascal; Schlegel, H Bernhard

    2015-06-04

    The angle-dependence of strong field ionization of O2, N2, CO2, and CH2O has been studied theoretically using a time-dependent configuration interaction approach with a complex absorbing potential (TDCIS-CAP). Calculation of the ionization yields as a function of the direction of polarization of the laser pulse produces three-dimensional surfaces of the angle-dependent ionization probability. These three-dimensional shapes and their variation with laser intensity can be interpreted in terms of ionization from the highest occupied molecular orbital (HOMO) and lower lying orbitals, and the Dyson orbitals for the ground and excited states of the cations.

  9. Helicity reversion in high-order-harmonic generation driven by bichromatic counter-rotating circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaofan; Li, Liang; Zhu, Xiaosong; Liu, Xi; Zhang, Qingbin; Lan, Pengfei; Lu, Peixiang

    2016-11-01

    We investigate the polarization properties of high harmonics generated with the bichromatic counter-rotating circularly polarized (BCCP) laser fields by numerically solving the time-dependent Schrödinger equation (TDSE). It is found that the helicity of the elliptically polarized harmonic emission is reversed at particular harmonic orders. Based on the time-frequency analysis and the classical three-step model, the correspondence between the positions of helicity reversions and the classical trajectories of continuum electrons is established. It is shown that the electrons ionized at one lobe of laser field can be divided into different groups based on the different lobes they recombine at, and the harmonics generated by adjacent groups have opposite helicities. Our study performs a detailed analysis of high harmonics in terms of electron trajectories and depicts a clear and intuitive physical picture of the HHG process in BCCP laser fields.

  10. Conduction band population in graphene in ultrashort strong laser field: Case of massive Dirac particles

    NASA Astrophysics Data System (ADS)

    Ahmadi, Z.; Goudarzi, H.; Jafari, A.

    2016-05-01

    The Dirac-like quasiparticles in honeycomb graphene lattice are taken to possess a non-zero effective mass. The charge carriers involve to interact with a femtosecond strong laser pulse. Due to the scattering time of electrons in graphene (τ ≈10-100 fs), the one femtosecond optical pulse is used to establish the coherence effect and, consequently, it can be realized to use the time-dependent Schrödinger equation for electron coupled with strong electromagnetic field. Generalized wave vector of relativistic electrons interacting with electric field of laser pulse causes to obtain a time-dependent electric dipole matrix element. Using the coupled differential equations of a two-state system of graphene, the density of probability of population transition between valence (VB) and conduction bands (CB) of gapped graphene is calculated. In particular, the effect of bandgap energy on dipole matrix elements at the Dirac points and resulting CB population (CBP) is investigated. The irreversible electron dynamics is achieved when the optical pulse end. Increasing the energy gap of graphene results in decreasing the maximum CBP.

  11. Orientation effects in high-order harmonic generation of H2^+ subject to strong laser fields

    NASA Astrophysics Data System (ADS)

    Telnov, Dmitry A.; Chu, Shih-I.

    2008-05-01

    We present ab initio 3D calculations of the orientation-dependent high-order harmonic generation (HHG) of the hydrogen molecular ion H2^+ subject to intense linearly polarized laser pulses with the wavelength 800nm [1]. The nuclei are kept at the equilibrium separation of 2 a.u., and the initial electronic state can be either 1σg (ground) or 1σu (first excited) state. Split-operator technique in the energy represenation and generalized pseudospectral discretization in prolate spheroidal coordinates are used to solve the time-dependent Schr"odinger equation. HHG power spectra show strong dependence on the orientation angle between the molecular axis and the polarization direction of the laser field. Particularly, orientation-selected resonances with other electronic states are well pronounced. Two-center interference effects in the HHG spectra are also analyzed.1. D. A. Telnov and S. I. Chu, Phys. Rev. A 76, 043412 (2007).

  12. Strong-field physics with mid-infrared lasers

    NASA Astrophysics Data System (ADS)

    Pogorelsky, I. V.

    2002-04-01

    Mid-infrared gas laser technology promises to become a unique tool for research in strong-field relativistic physics. The degree to which physics is relativistic is determined by a ponderomotive potential. At a given intensity, a 10 μm wavelength CO2 laser reaches a 100 times higher ponderomotive potential than the 1 μm wavelength solid state lasers. Thus, we can expect a proportional increase in the throughput of such processes as laser acceleration, x-ray production, etc. These arguments have been confirmed in proof-of-principle Thomson scattering and laser acceleration experiments conducted at BNL and UCLA where the first terawatt-class CO2 lasers are in operation. Further more, proposals for the 100 TW, 100 fs CO2 lasers based on frequency-chirped pulse amplification have been conceived. Such lasers can produce physical effects equivalent to a hypothetical multi-petawatt solid state laser. Ultra-fast mid-infrared lasers will open new routes to the next generation electron and ion accelerators, ultra-bright monochromatic femtosecond x-ray and gamma sources, allow to attempt the study of Hawking-Unruh radiation, and explore relativistic aspects of laser-matter interactions. We review the present status and experiments with terawatt-class CO2 lasers, sub-petawatt projects, and prospective applications in strong-field science. .

  13. Time-Dependent Interfacial Properties and DNAPL Mobility

    SciTech Connect

    Tuck, D.M.

    1999-03-10

    Interfacial properties play a major role in governing where and how dense nonaqueous phase liquids (DNAPLs) move in the subsurface. Interfacial tension and contact angle measurements were obtained for a simple, single component DNAPL (tetrachloroethene, PCE), complex laboratory DNAPLs (PCE plus Sudan IV dye), and a field DNAPL from the Savannah River Site (SRS) M-Area DNAPL (PCE, trichloroethene [TCE], and maching oils). Interfacial properties for complex DNAPLs were time-dependent, a phenomenon not observed for PCE alone. Drainage capillary pressure-saturation curves are strongly influenced by interfacial properties. Therefore time-dependence will alter the nature of DNAPL migration and penetration. Results indicate that the time-dependence of PCE with relatively high Sudan IV dye concentrations is comparable to that of the field DNAPL. Previous DNAPL mobility experiments in which the DNAPL was dyed should be reviewed to determine whether time-dependent properties influenced the resutls. Dyes appear to make DNAPL more complex, and therefore a more realistic analog for field DNAPLs than single component DNAPLs.

  14. Noncommutative quantum mechanics in a time-dependent background

    NASA Astrophysics Data System (ADS)

    Dey, Sanjib; Fring, Andreas

    2014-10-01

    We investigate a quantum mechanical system on a noncommutative space for which the structure constant is explicitly time dependent. Any autonomous Hamiltonian on such a space acquires a time-dependent form in terms of the conventional canonical variables. We employ the Lewis-Riesenfeld method of invariants to construct explicit analytical solutions for the corresponding time-dependent Schrödinger equation. The eigenfunctions are expressed in terms of the solutions of variants of the nonlinear Ermakov-Pinney equation and discussed in detail for various types of background fields. We utilize the solutions to verify a generalized version of Heisenberg's uncertainty relations for which the lower bound becomes a time-dependent function of the background fields. We study the variance for various states, including standard Glauber coherent states with their squeezed versions and Gaussian Klauder coherent states resembling a quasiclassical behavior. No type of coherent state appears to be optimal in general with regard to achieving minimal uncertainties, as this feature turns out to be background field dependent.

  15. Time-dependent freezing rate parcel model

    NASA Astrophysics Data System (ADS)

    Vali, G.; Snider, J. R.

    2015-02-01

    The time-dependent freezing rate (TDFR) model here described represents the formation of ice particles by immersion freezing within an air parcel. The air parcel trajectory follows an adiabatic ascent and includes a period in time when the parcel remains stationary at the top of its ascent. The description of the ice nucleating particles (INPs) in the air parcel is taken from laboratory experiments with cloud and precipitation samples and is assumed to represent the INP content of the cloud droplets in the parcel. Time dependence is included to account for variations in updraft velocity and for the continued formation of ice particles under isothermal conditions. The magnitudes of these factors are assessed on the basis of laboratory measurements. Results show that both factors give rise to three-fold variations in ice concentration for a realistic range of the input parameters. Refinements of the parameters specifying time dependence and INP concentrations are needed to make the results more specific to different atmospheric aerosol types. The simple model framework described in this paper can be adapted to more elaborate cloud models. The results here presented can help guide decisions on whether to include a time-dependent ice nucleation scheme or a simpler singular description in models.

  16. Time-dependent freezing rate parcel model

    NASA Astrophysics Data System (ADS)

    Vali, G.; Snider, J. R.

    2014-11-01

    The Time-Dependent Freezing Rate (TDFR) model here described represents the formation of ice particles by immersion freezing within an air parcel. The air parcel trajectory follows an adiabatic ascent and includes a period at time with the parcel remaining stationary at the top of its ascent. The description of the ice nucleating particles (INPs) in the air parcel is taken from laboratory experiments with cloud and precipitation samples and is assumed to represent the INP content of the cloud droplets in the parcel. Time-dependence is included to account for variations in updraft velocity and for the continued formation of ice particles at isothermal conditions. The magnitudes of these factors are assessed on the basis of laboratory measurements. Results show that both factors give rise to factors of about 3 variations in ice concentration for a realistic range of the input parameters. Refinements of the parameters specifying time-dependence and INP concentrations are needed to make the results more specific to different atmospheric aerosol types. The simple model framework described in this paper can be adapted to more elaborate cloud models. The results here presented can help guide decisions on whether to include a time-dependent ice nucleation scheme or a simpler singular description in models.

  17. Eigenfunction expansions for time dependent hamiltonians

    NASA Astrophysics Data System (ADS)

    Jauslin, H. R.; Guerin, S.; Deroussiaux, A.

    We describe a generalization of Floquet theory for non periodic time dependent Hamiltonians. It allows to express the time evolution in terms of an expansion in eigenfunctions of a generalized quasienergy operator. We discuss a conjecture on the extension of the adiabatic theorem to this type of systems, which gives a procedure for the physical preparation of Floquet states. *** DIRECT SUPPORT *** A3418380 00004

  18. R-matrix-incorporating-time theory of one-electron atomic and molecular systems in intense laser fields

    NASA Astrophysics Data System (ADS)

    Broin, Cathal Ó.; Nikolopoulos, L. A. A.

    2017-02-01

    In this thesis tutorial we discuss the R-matrix-incorporating-time ab initio theoretical framework for the solution of the time-dependent Schrödinger equation of one-electron atomic and molecular systems under strong electromagnetic fields. Within this approach, a division-of-space method is developed with the configuration space of the electron’s coordinates separated over two regions, the inner and outer regions. In the inner region the quantum system’s time-dependent wavefunction is expanded on the eigenstate basis set of its field-free Hamiltonian representation while in the outer region its grid representation is considered. The present tutorial describes in detail the theoretical formulation for one-electron quantum systems. Example calculations are discussed for atomic hydrogen, H, and the molecular hydrogen ion, {{{H}}}2+, in intense laser fields.

  19. Quasinormal modes in a time-dependent black hole background

    SciTech Connect

    Shao Chenggang; Wang Bin; Abdalla, Elcio; Su Rukeng

    2005-02-15

    We have studied the evolution of the massless scalar field propagating in a time-dependent charged Vaidya black hole background. A generalized tortoise coordinate transformation was used to study the evolution of the massless scalar field. It is shown that, for the slowest damped quasinormal modes, the approximate formulas in the stationary Reissner-Nordstroem black hole turn out to be a reasonable prescription, showing that results from quasinormal mode analysis are rather robust.

  20. Rapid Proton Transfer Mediated by a Strong Laser Field

    SciTech Connect

    Markevitch, Alexei N.; Levis, Robert J.; Romanov, Dmitri A.; Smith, Stanley M.

    2006-04-28

    Kinetic energy distributions of H{sup +} ejected from a polyatomic molecule, anthraquinone, subjected to 60 fs, 800 nm laser pulses of intensity between 0.2 and 4.0x10{sup 14} W{center_dot}cm{sup -2}, reveal field-driven restructuring of the molecule prior to Coulomb explosion. Calculations demonstrate fast intramolecular proton migration into a field-dressed metastable potential energy minimum. The proton migration occurs in the direction perpendicular to the polarization of the laser field. Rapid field-mediated isomerization is an important new phenomenon in coupling of polyatomic molecules with intense lasers.

  1. GAS LASERS FOR STRONG-FIELD APPLICATIONS.

    SciTech Connect

    POGORELSKY,I.V.

    2004-09-15

    Atomic-, molecular- and excimer-gas lasers employ variety of pumping schemes including electric discharge, optical, or chemical reactions and cover a broad spectral range from UV to far-IR. Several types of gas lasers can produce multi-kilojoule pulses and kilowatts of average power. Among them, excimer- and high-pressure molecular lasers have sufficient bandwidth for generating pico- and femtosecond pulses. Projects are underway and prospects are opening up to bring ultrafast gas laser technology to the front lines of advanced accelerator applications.

  2. Amplification of Relativistic Electron Bunches by Acceleration in Laser Fields

    NASA Astrophysics Data System (ADS)

    Braenzel, J.; Andreev, A. A.; Abicht, F.; Ehrentraut, L.; Platonov, K.; Schnürer, M.

    2017-01-01

    Direct acceleration of electrons in a coherent, intense light field is revealed by a remarkable increase of the electron number in the MeV energy range. Laser irradiation of thin polymer foils with a peak intensity of ˜1 ×1020 W /cm2 releases electron bunches along the laser propagation direction that are postaccelerated in the partly transmitted laser field. They are decoupled from the laser field at high kinetic energies, when a second foil target at an appropriate distance prevents their subsequent deceleration in the declining laser field. The scheme is established with laser pulses of high temporal contrast (1010 peak to background ratio) and two ultrathin polymer foils at a distance of 500 μ m . 2D particle in cell simulations and an analytical model confirm a significant change of the electron spectral distribution due to the double foil setup, which leads to an amplification of about 3 times of the electron number around a peak at 1 MeV electron energy. The result verifies a theoretical concept of direct electron bunch acceleration in a laser field that is scalable to extreme acceleration potential gradients. This method can be used to enhance the density and energy spread of electron bunches injected into postaccelerator stages of laser driven radiation sources.

  3. Solid state lasers for field application

    NASA Astrophysics Data System (ADS)

    Motenko, Boris N.; Ermakov, Boris A.; Berezin, Boris

    1991-03-01

    Lazer heads without forced cooling and of simple design used phosphate neodymium glass of laser rods for pulse rangfinders have been investigated.The headsensure laser performance for 20 years under adverse climatic conditions (t+50 C, relative humiditi of 98%) with an operating time of 4.10

  4. On time-dependent radiative transfer

    NASA Technical Reports Server (NTRS)

    Streater, A.; Cooper, J.; Sandle, W.

    1987-01-01

    An integral equation is developed for application to time-dependent laboratory experiments in which partial redistribution effects are important. The equation of transport with the Heasly-Kneer (1976) emission coefficient and the equation of statistical equilibrium lead to a time-dependent redistribution function containing an absorption - reemission term which decays exponentially in time and a scattering term which is instantaneous. This integral equation does not agree with an equation written by Payne et al. (1974) that has been used to compare theory with experiments. The difference between the Payne equation and the equation developed here needs to be examined in detail, since it might under some circumstances be on the same order as the difference between partial and complete redistribution.

  5. On time-dependent radiative transfer

    NASA Astrophysics Data System (ADS)

    Streater, A.; Cooper, J.; Sandle, W.

    1987-02-01

    An integral equation is developed for application to time-dependent laboratory experiments in which partial redistribution effects are important. The equation of transport with the Heasly-Kneer (1976) emission coefficient and the equation of statistical equilibrium lead to a time-dependent redistribution function containing an absorption - reemission term which decays exponentially in time and a scattering term which is instantaneous. This integral equation does not agree with an equation written by Payne et al. (1974) that has been used to compare theory with experiments. The difference between the Payne equation and the equation developed here needs to be examined in detail, since it might under some circumstances be on the same order as the difference between partial and complete redistribution.

  6. Time-Dependent Erosion of Ion Optics

    NASA Technical Reports Server (NTRS)

    Wirz, Richard E.; Anderson, John R.; Katz, Ira; Goebel, Dan M.

    2008-01-01

    The accurate prediction of thruster life requires time-dependent erosion estimates for the ion optics assembly. Such information is critical to end-of-life mechanisms such as electron backstreaming. CEX2D was recently modified to handle time-dependent erosion, double ions, and multiple throttle conditions in a single run. The modified code is called "CEX2D-t". Comparisons of CEX2D-t results with LDT and ELT post-tests results show good agreement for both screen and accel grid erosion including important erosion features such as chamfering of the downstream end of the accel grid and reduced rate of accel grid aperture enlargement with time.

  7. Time-dependent species sensitivity distributions.

    PubMed

    Fox, David R; Billoir, Elise

    2013-02-01

    Time is a central component of toxicity assessments. However, current ecotoxicological practice marginalizes time in concentration-response (C-R) modeling and species sensitivity distribution (SSD) analyses. For C-R models, time is invariably fixed, and toxicity measures are estimated from a function fitted to the data at that time. The estimated toxicity measures are used as inputs to the SSD modeling phase, which similarly avoids explicit recognition of the temporal component. The present study extends some commonly employed probability models for SSDs to derive theoretical results that characterize the time-dependent nature of hazardous concentration (HCx) values. The authors' results show that even from very simple assumptions, more complex patterns in the SSD time dependency can be revealed.

  8. Time-dependent oral absorption models

    NASA Technical Reports Server (NTRS)

    Higaki, K.; Yamashita, S.; Amidon, G. L.

    2001-01-01

    The plasma concentration-time profiles following oral administration of drugs are often irregular and cannot be interpreted easily with conventional models based on first- or zero-order absorption kinetics and lag time. Six new models were developed using a time-dependent absorption rate coefficient, ka(t), wherein the time dependency was varied to account for the dynamic processes such as changes in fluid absorption or secretion, in absorption surface area, and in motility with time, in the gastrointestinal tract. In the present study, the plasma concentration profiles of propranolol obtained in human subjects following oral dosing were analyzed using the newly derived models based on mass balance and compared with the conventional models. Nonlinear regression analysis indicated that the conventional compartment model including lag time (CLAG model) could not predict the rapid initial increase in plasma concentration after dosing and the predicted Cmax values were much lower than that observed. On the other hand, all models with the time-dependent absorption rate coefficient, ka(t), were superior to the CLAG model in predicting plasma concentration profiles. Based on Akaike's Information Criterion (AIC), the fluid absorption model without lag time (FA model) exhibited the best overall fit to the data. The two-phase model including lag time, TPLAG model was also found to be a good model judging from the values of sum of squares. This model also described the irregular profiles of plasma concentration with time and frequently predicted Cmax values satisfactorily. A comparison of the absorption rate profiles also suggested that the TPLAG model is better at prediction of irregular absorption kinetics than the FA model. In conclusion, the incorporation of a time-dependent absorption rate coefficient ka(t) allows the prediction of nonlinear absorption characteristics in a more reliable manner.

  9. Dissipative time-dependent quantum transport theory.

    PubMed

    Zhang, Yu; Yam, Chi Yung; Chen, GuanHua

    2013-04-28

    A dissipative time-dependent quantum transport theory is developed to treat the transient current through molecular or nanoscopic devices in presence of electron-phonon interaction. The dissipation via phonon is taken into account by introducing a self-energy for the electron-phonon coupling in addition to the self-energy caused by the electrodes. Based on this, a numerical method is proposed. For practical implementation, the lowest order expansion is employed for the weak electron-phonon coupling case and the wide-band limit approximation is adopted for device and electrodes coupling. The corresponding hierarchical equation of motion is derived, which leads to an efficient and accurate time-dependent treatment of inelastic effect on transport for the weak electron-phonon interaction. The resulting method is applied to a one-level model system and a gold wire described by tight-binding model to demonstrate its validity and the importance of electron-phonon interaction for the quantum transport. As it is based on the effective single-electron model, the method can be readily extended to time-dependent density functional theory.

  10. Time Dependent Behavior in the Weissenberg Effect

    NASA Astrophysics Data System (ADS)

    Degen, Michael M.; Andereck, C. David

    1997-03-01

    The Weissenberg effect is the climb of a non-Newtonian fluid up a rotating rod. We have found novel transitional effects in the behavior of a particular climbing fluid, STP(STP Oil Treatment distributed by First Brands Corporation.). The first state is a time-independent axisymmetric concave climb. As the rotation rate of the rod is increased, the first transition is to an axisymmetric climb with an ``onion dome'' shape. At higher rotation rates, the flow undergoes a symmetry breaking bifurcation to a time-dependent state. This time-dependent state exhibits an oscillation with a single frequency. Upon further increase of the rod rotation rate, the oscillation becomes modulated by a second frequency. The nature of each transition will be characterized, including the measurement of oscillation amplitudes and the frequency (or frequencies) of the time dependent states. These results will be compared with previous work.(G.S. Beavers, D.D. Joseph, J. Fluid Mech. 69), 475 (1975).(D.D. Joseph, R.L. Fosdick, Arch. Rational Mech. 49), 321 (1973).

  11. Magnetic Field Generation and Electron Acceleration in Relativistic Laser Channel

    SciTech Connect

    I.Yu. Kostyukov; G. Shvets; N.J. Fisch; J.M. Rax

    2001-12-12

    The interaction between energetic electrons and a circularly polarized laser pulse inside an ion channel is studied. Laser radiation can be resonantly absorbed by electrons executing betatron oscillations in the ion channel and absorbing angular momentum from the laser. The absorbed angular momentum manifests itself as a strong axial magnetic field (inverse Faraday effect). The magnitude of this magnetic field is calculated and related to the amount of the absorbed energy. Absorbed energy and generated magnetic field are estimated for the small and large energy gain regimes. Qualitative comparisons with recent experiments are also made.

  12. Temperature field modeling in laser-heated metals for laser cleaning of surfaces

    NASA Astrophysics Data System (ADS)

    Oane, Mihai; Apostol, Ileana; Timcu, Adrian

    2003-10-01

    Laser induced surface cleaning is the adequate method in a large variety of industrial domains as microelectronics, optics, photonics. By comparison to chemical and/or mechanical cleaning, laser cleaning has the advantage of a very good selectivity on the surface and in depth of the material, no surface contamination, without stress in the material volume and environmental safe. It seems that laser cleaning can be developed in a method to be currently used in microelectronic industry. For an efficient laser cleaning of metallic thin films without damage of the silicon wafer, a careful optimization of the incident laser energy, fluence, intensity and number of laser pulses is needed. We have developed an analytical procedure to study the temperature fields in pulsed laser heated solids, for a deeper knowledge of the laser-thin film substrate interaction.

  13. Multiphoton and tunneling ionization probability of atoms and molecules in an intense laser field

    NASA Astrophysics Data System (ADS)

    Zhao, Song-Feng; Liu, Lu; Zhou, Xiao-Xin

    2014-02-01

    We theoretically studied ionization of atoms exposed to an intense laser field by using three different methods, i.e., the numerical solution of the single-active-electron approximation based time-dependent Schrödinger equation (SAE-TDSE), the Perelomov-Popov-Terent'ev (PPT) model, and the Ammosov-Delone-Krainov (ADK) model. The ionization of several linear molecules in a strong laser field is also investigated with the molecular ADK (MO-ADK) and the molecular PPT (MO-PPT) model. We show that the ionization probability from the PPT and the MO-PPT model agrees well with the corresponding SAE-TDSE result in both the multiphoton and tunneling ionization regimes. By considering the volume effect of the laser field, the ionization signal obtained from the PPT and the MO-PPT model fits well the experimental data in the whole range of the multiphoton and tunneling ionization regimes. However, both the ADK and MO-ADK models seriously underestimate the ionization probabilities (or signals) in the multiphoton regime.

  14. Mechanism of enhanced ionization of linear H+3 in intense laser fields

    NASA Astrophysics Data System (ADS)

    Kawata, I.; Kono, H.; Bandrauk, A. D.

    2001-10-01

    We investigate the mechanism of enhanced ionization that occurs at a critical internuclear distance Rc in the two-electron symmetric linear triatomic molecule H+3 subjected to an ultrashort, intense laser pulse by solving exactly the time-dependent Schrödinger equation for a one-dimensional model of H+3. Results of the simulations are analyzed by using three essential adiabatic field states \\|1>, \\|2>, and \\|3> that are adiabatically connected with the lowest three electronic states X1Σ+g, B1Σ+u, and E1Σ+g of the field free ion. We give also a simple MO (molecular orbital) picture in terms of these three states to illustrate the important electronic configurations in an intense field. The states \\|1>, \\|2>, and \\|3> are shown to be composed mainly of the configurations HHH+, HH+H, and H+HH, respectively in the presence of the field. We conclude that the overall level dynamics is governed mainly by transitions at the zero-field energy quasicrossings of these three states. The response of H+3 to a laser field can be classified into two regimes. In the adiabatic regime (RRc), internuclear electron transfer is suppressed due to electron repulsion and laser induced localization. In the intermediate (R~=Rc) region, where enhanced ionization occurs, the state \\|3> is most efficiently created by the field-induced nonadiabatic transitions between the states at quasicrossing points. The ``quasistatic'' laser-induced potential barriers are low enough for the electron to tunnel from the ascending (upper) well, thus confirming the quasistatic model at high intensities. Analytic expressions for the critical distance Rc are obtained from this model and collective electron motion is inferred from the detailed time-dependent two-electron distributions.

  15. Coherent destruction of tunneling in a six-dimensional model of NHD2: A computational study using the multi-configuration time-dependent Hartree method

    NASA Astrophysics Data System (ADS)

    Sala, Matthieu; Gatti, Fabien; Guérin, Stéphane

    2014-10-01

    We investigate the phenomenon of coherent destruction of tunneling in a six-dimensional model of the NHD2 molecule. Two regimes are considered for the frequency of the laser field. A non-resonant regime where the frequency of the laser field is high with respect to the ground vibrational state tunneling splitting but smaller than the transition frequencies between the ground and excited vibrational states; and a quasi-resonant regime where the frequency of the laser field is close to the transition frequency between the ground and first excited vibrational states. In each case, we study the laser driven dynamics in the framework of the Floquet formalism and derive simple analytical formulas that explain the shape of the quasienergy curves associated with the two tunneling components of the ground vibrational state. This analysis allows us to obtain the parameters (frequency and amplitude) of the laser field that lead to the coherent destruction of tunneling. The multi-configuration time-dependent Hartree method is then used to solve the time-dependent Schrödinger equation for a six-dimensional model of the molecule in interaction with an adiabatically turned on monochromatic laser field, in order to confirm the results obtained from this analysis.

  16. Time-dependent local density measurements in unsteady flows

    NASA Technical Reports Server (NTRS)

    Mckenzie, R. L.; Monson, D. J.; Exberger, R. J.

    1979-01-01

    A laser-induced fluorescence technique for measuring the relative time-dependent density fluctuations in unsteady or turbulent flows is demonstrated. Using a 1.5-W continuous-wave Kr(+) laser, measurements have been obtained in 0.1-mm diameter by 1-mm-long sampling volumes in a Mach 3 flow of N2 seeded with biacetyl vapor. A signal amplitude resolution of 2% was achieved for a detection frequency bandwidth of 10 kHz. The measurement uncertainty was found to be dominated by noise behaving as photon statistical noise. The practical limits of signal-to-noise ratios have been characterized for a wide range of detection frequency bandwidths that encompasses those of interest in supersonic turbulence measurements.

  17. Nonadiabatic Electron Dynamics in Orthogonal Two-Color Laser Fields with Comparable Intensities.

    PubMed

    Geng, Ji-Wei; Xiong, Wei-Hao; Xiao, Xiang-Ru; Peng, Liang-You; Gong, Qihuang

    2015-11-06

    We theoretically investigate the nonadiabatic subcycle electron dynamics in orthogonally polarized two-color laser fields with comparable intensities. The photoelectron dynamics is simulated by exact solution to the 3D time-dependent Schrödinger equation, and also by two other semiclassical methods, i.e., the quantum trajectory Monte Carlo simulation and the Coulomb-corrected strong field approximation. Through these methods, we identify the underlying mechanisms of the subcycle electron dynamics and find that both the nonadiabatic effects and the Coulomb potential play very important roles. The contribution of the nonadiabatic effects manifest in two aspects, i.e., the nonadiabatic ionization rate and the nonzero initial velocities at the tunneling exit. The Coulomb potential has a different impact on the electrons' trajectories for different relative phases between the two pulses.

  18. Effect of transverse magnetic field on laser produced plasma expansion into vacuum

    SciTech Connect

    Bennaceur-Doumaz, D.; Djebli, M.

    2011-08-15

    A one-dimensional time-dependent magneto-hydrodynamic ideal model is used to investigate the dynamics of initially magnetized laser produced plasma expansion into vacuum, in the context of inertial fusion. The plasma is assumed to be fully ionized and in local thermodynamic equilibrium (LTE), allowing all charged particles to have the same temperatures. Self-similar solution shows that the density, velocity, and temperature increase with the strength of the magnetic field. The transverse magnetic field causes significant changes in the plasma expansion dynamics, including the plasma confinement. The plasma velocity increasing is also observed and the temperature is found to be larger compared to temperature in un-magnetized case.

  19. Jet methods in time-dependent Lagrangian biomechanics

    NASA Astrophysics Data System (ADS)

    Ivancevic, Tijana T.

    2010-10-01

    In this paper we propose the time-dependent generalization of an ‘ordinary’ autonomous human biomechanics, in which total mechanical + biochemical energy is not conserved. We introduce a general framework for time-dependent biomechanics in terms of jet manifolds associated to the extended musculo-skeletal configuration manifold, called the configuration bundle. We start with an ordinary configuration manifold of human body motion, given as a set of its all active degrees of freedom (DOF) for a particular movement. This is a Riemannian manifold with a material metric tensor given by the total mass-inertia matrix of the human body segments. This is the base manifold for standard autonomous biomechanics. To make its time-dependent generalization, we need to extend it with a real time axis. By this extension, using techniques from fibre bundles, we defined the biomechanical configuration bundle. On the biomechanical bundle we define vector-fields, differential forms and affine connections, as well as the associated jet manifolds. Using the formalism of jet manifolds of velocities and accelerations, we develop the time-dependent Lagrangian biomechanics. Its underlying geometric evolution is given by the Ricci flow equation.

  20. Jet methods in time-dependent Lagrangian biomechanics

    NASA Astrophysics Data System (ADS)

    Ivancevic, Tijana

    2010-10-01

    In this paper we propose the time-dependent generalization of an `ordinary' autonomous human biomechanics, in which total mechanical + biochemical energy is not conserved. We introduce a general framework for time-dependent biomechanics in terms of jet manifolds associated to the extended musculo-skeletal configuration manifold, called the configuration bundle. We start with an ordinary configuration manifold of human body motion, given as a set of its all active degrees of freedom (DOF) for a particular movement. This is a Riemannian manifold with a material metric tensor given by the total mass-inertia matrix of the human body segments. This is the base manifold for standard autonomous biomechanics. To make its time-dependent generalization, we need to extend it with a real time axis. By this extension, using techniques from fibre bundles, we defined the biomechanical configuration bundle. On the biomechanical bundle we define vector-fields, differential forms and affine connections, as well as the associated jet manifolds. Using the formalism of jet manifolds of velocities and accelerations, we develop the time-dependent Lagrangian biomechanics. Its underlying geometric evolution is given by the Ricci flow equation.

  1. Xenon clusters in intense VUV laser fields.

    PubMed

    Santra, Robin; Greene, Chris H

    2003-12-05

    A simple model is developed that quantitatively describes intense interactions of a vacuum ultraviolet (VUV) laser pulse with a xenon cluster. We find good agreement with a recent experiment [Nature (London) 420, 482 (2002)

  2. Time-dependent Hartree approximation and time-dependent harmonic oscillator model

    NASA Astrophysics Data System (ADS)

    Blaizot, J. P.; Schulz, H.

    1982-03-01

    We present an analytically soluble model for studying nuclear collective motion within the framework of the time-dependent Hartree (TDH) approximation. The model reduces the TDH equations to the Schrödinger equation of a time-dependent harmonic oscillator. Using canonical transformations and coherent states we derive a few properties of the time-dependent harmonic oscillator which are relevant for applications. We analyse the role of the normal modes in the time evolution of a system governed by TDH equations. We show how these modes couple together due to the anharmonic terms generated by the non-linearity of the theory.

  3. Time-Dependent 5D Solutions of the Einstein Equations

    SciTech Connect

    Lopez, L. A.

    2010-07-12

    In this work are obtained 5D time-dependent solutions of Einstein equations, one is obtained by means of equiping a cylindrically symmetry solution (JEKK) with a scalar field, then lifting it to a fifth dimension. The other is obtained transforming the Myers-Perry solution via Wick rotation. The two solutions can be interpreted as gravitational waves in some cases. The singularities and C-energy are addressed.

  4. Generation of quasistationary magnetic fields in a turbulent laser plasma

    NASA Astrophysics Data System (ADS)

    Bychenkov, V. Iu.; Gradov, O. M.; Chokparova, G. A.

    1984-07-01

    A theory is derived for the generation of quasi-stationary magnetic fields in a laser plasma with well developed ion-acoustic turbulence. Qualitative changes are caused in the nature of the magnetic-field generation by an anomalous anisotropic transport in the turbulent plasma. The role played by turbulent diffusion and thermodiffusive transport in the magnetic-field saturation is discussed.

  5. Time-dependent Dyson orbital theory.

    PubMed

    Gritsenko, O V; Baerends, E J

    2016-08-21

    Although time-dependent density functional theory (TDDFT) has become the tool of choice for real-time propagation of the electron density ρ(N)(t) of N-electron systems, it also encounters problems in this application. The first problem is the neglect of memory effects stemming from the, in TDDFT virtually unavoidable, adiabatic approximation, the second problem is the reliable evaluation of the probabilities P(n)(t) of multiple photoinduced ionization, while the third problem (which TDDFT shares with other approaches) is the reliable description of continuum states of the electrons ejected in the process of ionization. In this paper time-dependent Dyson orbital theory (TDDOT) is proposed. Exact TDDOT equations of motion (EOMs) for time-dependent Dyson orbitals are derived, which are linear differential equations with just static, feasible potentials of the electron-electron interaction. No adiabatic approximation is used, which formally resolves the first TDDFT problem. TDDOT offers formally exact expressions for the complete evolution in time of the wavefunction of the outgoing electron. This leads to the correlated probability of single ionization P(1)(t) as well as the probabilities of no ionization (P(0)(t)) and multiple ionization of n electrons, P(n)(t), which formally solves the second problem of TDDFT. For two-electron systems a proper description of the required continuum states appears to be rather straightforward, and both P(1)(t) and P(2)(t) can be calculated. Because of the exact formulation, TDDOT is expected to reproduce a notorious memory effect, the "knee structure" of the non-sequential double ionization of the He atom.

  6. Time-Dependent Protein Thermostability Assay.

    PubMed

    Vandecaetsbeek, Ilse; Vangheluwe, Peter

    2016-01-01

    Membrane protein purification often yields rather unstable proteins impeding functional and structural protein characterization. Low protein stability also leads to low purification yields as a result of protein degradation, aggregation, precipitation, and folding instability. It is often required to optimize buffer conditions through numerous iterations of trial and error to improve the homogeneity, stability, and solubility of the protein sample demanding high amounts of purified protein. Therefore we have set up a fast, simple, and high-throughput time-dependent thermostability-based assay at low protein cost to identify protein stabilizing factors to facilitate the handling and characterization of membrane proteins by subsequent structural and functional studies.

  7. A Time Dependent Transport Equation Solver

    DTIC Science & Technology

    1991-05-01

    Using TWIGL Mesh Spacing ............. 63 11 Initial FEMP2D Flux Using 2X TWIGL Mesh Spacing ........ .. 64 12 Time Dependent Thermal Absorption...energy group, and g = G is the lowest ( thermal ) energy group. ?oo(r, E, t) the coefficient in the P approximation that phys- ically r’iDresents the total...than these MrPs. This suggest that the thermal flux calculations could be suspect. Indeed, both the FEMP2D and FMP2DT calculations showed that the

  8. Eisenhart lifts and symmetries of time-dependent systems

    NASA Astrophysics Data System (ADS)

    Cariglia, M.; Duval, C.; Gibbons, G. W.; Horváthy, P. A.

    2016-10-01

    Certain dissipative systems, such as Caldirola and Kannai's damped simple harmonic oscillator, may be modelled by time-dependent Lagrangian and hence time dependent Hamiltonian systems with n degrees of freedom. In this paper we treat these systems, their projective and conformal symmetries as well as their quantisation from the point of view of the Eisenhart lift to a Bargmann spacetime in n + 2 dimensions, equipped with its covariantly constant null Killing vector field. Reparametrisation of the time variable corresponds to conformal rescalings of the Bargmann metric. We show how the Arnold map lifts to Bargmann spacetime. We contrast the greater generality of the Caldirola-Kannai approach with that of Arnold and Bateman. At the level of quantum mechanics, we are able to show how the relevant Schrödinger equation emerges naturally using the techniques of quantum field theory in curved spacetimes, since a covariantly constant null Killing vector field gives rise to well defined one particle Hilbert space. Time-dependent Lagrangians arise naturally also in cosmology and give rise to the phenomenon of Hubble friction. We provide an account of this for Friedmann-Lemaître and Bianchi cosmologies and how it fits in with our previous discussion in the non-relativistic limit.

  9. Electron-atom collisions in a laser field

    NASA Astrophysics Data System (ADS)

    Smith, Philip H. G.; Flannery, M. R.

    1991-05-01

    Cross sections tor the 1S-2S and 1S-2P 0 transitions in laser assisted e-H(1S) collisions are calculated in both the multichannel eikonal and the Born-wave treatments as a function of impact energy and laser field intensity and phase. The laser considered is a monotonic, plane polarized CO 2 laser (photon energy = 0.117 eV), with the polarization direction parallel to the initial projectile velocity. Floquet dressing of the hydrogen atom in the soft-photon weak-field limit reveals a concise description of the laser assisted electron-atom collision. This model also links the microscopic detail of the individual collisions with the macroscopic considerations of experimental analysis.

  10. Atomic excitation and acceleration in strong laser fields

    NASA Astrophysics Data System (ADS)

    Zimmermann, H.; Eichmann, U.

    2016-10-01

    Atomic excitation in the tunneling regime of a strong-field laser-matter interaction has been recently observed. It is conveniently explained by the concept of frustrated tunneling ionization (FTI), which naturally evolves from the well-established tunneling picture followed by classical dynamics of the electron in the combined laser field and Coulomb field of the ionic core. Important predictions of the FTI model such as the n distribution of Rydberg states after strong-field excitation and the dependence on the laser polarization have been confirmed in experiments. The model also establishes a sound basis to understand strong-field acceleration of neutral atoms in strong laser fields. The experimental observation has become possible recently and initiated a variety of experiments such as atomic acceleration in an intense standing wave and the survival of Rydberg states in strong laser fields. Furthermore, the experimental investigations on strong-field dissociation of molecules, where neutral excited fragments after the Coulomb explosion of simple molecules have been observed, can be explained. In this review, we introduce the subject and give an overview over relevant experiments supplemented by new results.

  11. Time-Dependent SSC Cooling Effects on Blazar Emission

    NASA Astrophysics Data System (ADS)

    Zacharias, Michael; Schlickeiser, Reinhard

    2014-03-01

    Blazars are among the most violent sources in the cosmos exhibiting flaring states with remarkably different variability time scales. Especially rapid flares with flux doubling time scales of the order of minutes have been puzzling for quite some time. Many modeling attempts use the well known linear and steady-state scenario for the cooling and emission processes in the jet, albeit the obvious strongly time-dependent nature of flares. Due to the feedback of the self-produced synchrotron radiation with additional scattering by the relativistic electrons, the synchrotron-self Compton (SSC) effect is inherently time-dependent. Recently, an analytical analysis on the effects of this nonlinear behavior has been presented. Here, we summarize these results concerning the effect of the time-dependent SSC cooling on the spectral energy distribution (SED), and the synchrotron lightcurves of blazars. For that, we calculated analytically the synchrotron, SSC and external Compton (EC) component of the SED, giving remarkably different spectral features compared to the standard linear approach. The resulting fluxes strongly depend on the parameters, and SSC might have a strong effect even in sources with strong external photon fields (such as FSRQs). For the synchrotron lightcurve we considered the effects of retardation, including the geometry of the source. The retardation might smear out some effects of the time-dependent cooling, but since lightcurves and SEDs have to be fitted simultaneously with the same set of parameters, the results give nonetheless important clues about the source. Thus, we argue for a wide utilization of the time-dependent treatment in modeling (especially rapid) blazar flares, since it accounts for features in the SED and the lightcurves that are usually accounted for by introducing several breaks in the electron distribution without any physical justification.

  12. Electron Dynamics in Nanostructures in Strong Laser Fields

    SciTech Connect

    Kling, Matthias

    2014-09-11

    The goal of our research was to gain deeper insight into the collective electron dynamics in nanosystems in strong, ultrashort laser fields. The laser field strengths will be strong enough to extract and accelerate electrons from the nanoparticles and to transiently modify the materials electronic properties. We aimed to observe, with sub-cycle resolution reaching the attosecond time domain, how collective electronic excitations in nanoparticles are formed, how the strong field influences the optical and electrical properties of the nanomaterial, and how the excitations in the presence of strong fields decay.

  13. Measuring Energy Scaling of Laser Driven Magnetic Fields

    NASA Astrophysics Data System (ADS)

    Williams, Jackson; Goyon, Clement; Mariscal, Derek; Pollock, Brad; Patankar, Siddharth; Moody, John

    2016-10-01

    Laser-driven magnetic fields are of interest in particle confinement, fast ignition, and ICF platforms as an alternative to pulsed power systems to achieve many times higher fields. A comprehensive model describing the mechanism responsible for creating and maintaining magnetic fields from laser-driven coils has not yet been established. Understanding the scaling of key experimental parameters such as spatial and temporal uniformity and duration are necessary to implement coil targets in practical applications yet these measurements prove difficult due to the highly transient nature of the fields. We report on direct voltage measurements of laser-driven coil targets in which the laser energy spans more than four orders of magnitude. Results suggest that at low energies, laser-driven coils can be modeled as an electric circuit; however, at higher energies plasma effects dominate and a simple circuit treatment is insufficient to describe all observed phenomenon. The favorable scaling with laser power and pulse duration, observed in the present study and others at kilojoule energies, has positive implications for sustained, large magnetic fields for applications on the NIF. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  14. Time dependent deformation of Kilauea Volcano, Hawaii

    NASA Astrophysics Data System (ADS)

    Montgomery-Brown, Emily Kvietka Desmarais

    to a decollement structure 8 km under the south flank, and the locations of the microearthquakes suggest that both occur on the same structure. In 2007, Episode 56 of the Pu'u 'O'o-Kupianaha eruption occurred. This episode was exciting both because it was the largest intrusion in the last decade, and because it occurred concurrently with a flank slow-slip event. The intrusion started on Father's day (June 17th), 2007 with increased seismicity and abrupt tilts at the summit and rift zones. Quasi-static models of the total deformation determined from GPS, tilt, and InSAR indicate that the intrusion occurred on two en echelon dike segments in the upper East Rift Zone along with deformation consistent with slow-slip in the same areas of previous events. The ˜ 2 m maximum opening occurred on the eastern segment near Makaopui crater. Unlike previous intrusions in 1997, 1999, and 2000, the dike model was not sufficient to explain deformation on the western flank. Additionally, a coastal tiltmeter installed in anticipation of a slow-slip event recorded tilts consistent with those observed during the 2005 slow-slip event. These observations led to the conclusion that a concurrent slow-slip event occurred. Geodetic models indicate a similar amount of decollement slip occurred as in previous slow-slip events. Sub-daily GPS positions were used to study the spatio-temporal distribution of the dike intrusion. The time-dependent intrusion model shows that the intrusion began on the western en echelon segment before jumping to the eastern segment, which accumulated the majority of the 2 m of opening. Sub-daily GPS positions limit the number of stations available since there are very few continuous stations north of the East Rift Zone, where coverage is critical for separating the intrusion from the slow-slip. However, an ENVISAT interferogram at 08:22 on June 18, 2007 provides additional spatial coverage of deformation up to that point. Combining this image with the GPS and tilt

  15. Time-dependent magnetohydrodynamic simulations of the inner heliosphere

    NASA Astrophysics Data System (ADS)

    Merkin, V. G.; Lyon, J. G.; Lario, D.; Arge, C. N.; Henney, C. J.

    2016-04-01

    This paper presents results from a simulation study exploring heliospheric consequences of time-dependent changes at the Sun. We selected a 2 month period in the beginning of year 2008 that was characterized by very low solar activity. The heliosphere in the equatorial region was dominated by two coronal holes whose changing structure created temporal variations distorting the classical steady state picture of the heliosphere. We used the Air Force Data Assimilate Photospheric Flux Transport (ADAPT) model to obtain daily updated photospheric magnetograms and drive the Wang-Sheeley-Arge (WSA) model of the corona. This leads to a formulation of a time-dependent boundary condition for our three-dimensional (3-D) magnetohydrodynamic (MHD) model, LFM-helio, which is the heliospheric adaptation of the Lyon-Fedder-Mobarry MHD simulation code. The time-dependent coronal conditions were propagated throughout the inner heliosphere, and the simulation results were compared with the spacecraft located near 1 astronomical unit (AU) heliocentric distance: Advanced Composition Explorer (ACE), Solar Terrestrial Relations Observatory (STEREO-A and STEREO-B), and the MErcury Surface, Space ENvironment, GEochemistry, and Ranging (MESSENGER) spacecraft that was in cruise phase measuring the heliospheric magnetic field between 0.35 and 0.6 AU. In addition, during the selected interval MESSENGER and ACE aligned radially allowing minimization of the effects of temporal variation at the Sun versus radial evolution of structures. Our simulations show that time-dependent simulationsreproduce the gross-scale structure of the heliosphere with higher fidelity, while on smaller spatial and faster time scales (e.g., 1 day) they provide important insights for interpretation of the data. The simulations suggest that moving boundaries of slow-fast wind transitions at 0.1 AU may result in the formation of inverted magnetic fields near pseudostreamers which is an intrinsically time-dependent process

  16. Quantum control of multidimensional systems: Implementation within the time-dependent Hartree approximation

    NASA Astrophysics Data System (ADS)

    Messina, Michael; Wilson, Kent R.; Krause, Jeffrey L.

    1996-01-01

    The exact formulation of quantum control is now well known and sufficiently general to describe multidimensional quantum systems. The implementation of this formalism relies on the solution of the time-dependent Schrödinger equation (TDSE) of the system under study, and thus far has been limited for computational reasons to simple quantum systems of very small dimensionality. To study quantum control in larger systems, such as polyatomic molecules and condensed phases, we explore an implementation of the control formalism in which the TDSE is solved approximately using the time-dependent Hartree (TDH) approximation. We demonstrate formally that the TDH approximation greatly simplifies the implementation of control in the weak response regime for multidimensional systems. We also present numerical examples to show that the TDH approximation for the weak response case is sufficiently accurate to predict the laser fields that best drive a quantum system to a desired goal at a desired time, in systems containing more than one degree of freedom, by considering a two-dimensional quantum system and comparing the optimal fields obtained by solving the TDSE exactly to those obtained using the TDH approximation.

  17. Holonomic Quantum Computation by Time dependent Decoherence Free Subspaces

    NASA Astrophysics Data System (ADS)

    Lin, J. N.; Liang, Y.; Yang, H. D.; Gui, J.; Wu, S. L.

    2017-01-01

    We show how to realize nonadiabatic holonomic quantum computation in time-dependent decoherence free subspaces (TDFSs). In our scheme, the holonomy is not generated by computational bases in DFSs but time-dependent bases of TDFSs. Therefore, different from the traditional DFSs, the ancillary systems are not necessary in inducing holonomy, which saves qubits used in the holonomic quantum computation. We also analyze the symmetry of the N-qubits system which couples to a common squeezed field. The results show that, there are several independent DFSs presented in Hilbert space, which is determined by eigenvalues of Lindblad operators. Combining the scheme and the model proposed in this paper, we show that, the one-qubit controllable phase gate can be realized by only two physical qubits.

  18. Holonomic Quantum Computation by Time dependent Decoherence Free Subspaces

    NASA Astrophysics Data System (ADS)

    Lin, J. N.; Liang, Y.; Yang, H. D.; Gui, J.; Wu, S. L.

    2017-04-01

    We show how to realize nonadiabatic holonomic quantum computation in time-dependent decoherence free subspaces (TDFSs). In our scheme, the holonomy is not generated by computational bases in DFSs but time-dependent bases of TDFSs. Therefore, different from the traditional DFSs, the ancillary systems are not necessary in inducing holonomy, which saves qubits used in the holonomic quantum computation. We also analyze the symmetry of the N-qubits system which couples to a common squeezed field. The results show that, there are several independent DFSs presented in Hilbert space, which is determined by eigenvalues of Lindblad operators. Combining the scheme and the model proposed in this paper, we show that, the one-qubit controllable phase gate can be realized by only two physical qubits.

  19. Time-dependent Cooling in Photoionized Plasma

    NASA Astrophysics Data System (ADS)

    Gnat, Orly

    2017-02-01

    I explore the thermal evolution and ionization states in gas cooling from an initially hot state in the presence of external photoionizing radiation. I compute the equilibrium and nonequilibrium cooling efficiencies, heating rates, and ion fractions for low-density gas cooling while exposed to the ionizing metagalactic background radiation at various redshifts (z = 0 ‑ 3), for a range of temperatures (108–104 K), densities (10‑7–103 cm‑3), and metallicities (10‑3–2 times solar). The results indicate the existence of a threshold ionization parameter, above which the cooling efficiencies are very close to those in photoionization equilibrium (so that departures from equilibrium may be neglected), and below which the cooling efficiencies resemble those in collisional time-dependent gas cooling with no external radiation (and are thus independent of density).

  20. Determination of Time Dependent Virus Inactivation Rates

    NASA Astrophysics Data System (ADS)

    Chrysikopoulos, C. V.; Vogler, E. T.

    2003-12-01

    A methodology is developed for estimating temporally variable virus inactivation rate coefficients from experimental virus inactivation data. The methodology consists of a technique for slope estimation of normalized virus inactivation data in conjunction with a resampling parameter estimation procedure. The slope estimation technique is based on a relatively flexible geostatistical method known as universal kriging. Drift coefficients are obtained by nonlinear fitting of bootstrap samples and the corresponding confidence intervals are obtained by bootstrap percentiles. The proposed methodology yields more accurate time dependent virus inactivation rate coefficients than those estimated by fitting virus inactivation data to a first-order inactivation model. The methodology is successfully applied to a set of poliovirus batch inactivation data. Furthermore, the importance of accurate inactivation rate coefficient determination on virus transport in water saturated porous media is demonstrated with model simulations.

  1. Time-dependent landslide probability mapping

    USGS Publications Warehouse

    Campbell, Russell H.; Bernknopf, Richard L.; ,

    1993-01-01

    Case studies where time of failure is known for rainfall-triggered debris flows can be used to estimate the parameters of a hazard model in which the probability of failure is a function of time. As an example, a time-dependent function for the conditional probability of a soil slip is estimated from independent variables representing hillside morphology, approximations of material properties, and the duration and rate of rainfall. If probabilities are calculated in a GIS (geomorphic information system ) environment, the spatial distribution of the result for any given hour can be displayed on a map. Although the probability levels in this example are uncalibrated, the method offers a potential for evaluating different physical models and different earth-science variables by comparing the map distribution of predicted probabilities with inventory maps for different areas and different storms. If linked with spatial and temporal socio-economic variables, this method could be used for short-term risk assessment.

  2. High Magnetic field generation for laser-plasma experiments

    SciTech Connect

    Pollock, B B; Froula, D H; Davis, P F; Ross, J S; Fulkerson, S; Bower, J; Satariano, J; Price, D; Glenzer, S H

    2006-05-01

    An electromagnetic solenoid was developed to study the effect of magnetic fields on electron thermal transport in laser plasmas. The solenoid, which is driven by a pulsed power system suppling 30 kJ, achieves magnetic fields of 13 T. The field strength was measured on the solenoid axis with a magnetic probe and optical Zeeman splitting. The measurements agree well with analytical estimates. A method for optimizing the solenoid design to achieve magnetic fields exceeding 20 T is presented.

  3. Multipass laser amplification with near-field far-field optical separation

    DOEpatents

    Hagen, Wilhelm F.

    1979-01-01

    This invention discloses two classes of optical configurations for high power laser amplification, one allowing near-field and the other allowing far-field optical separation, for the multiple passage of laser pulses through one or more amplifiers over an open optical path. These configurations may reimage the amplifier or any other part of the cavity on itself so as to suppress laser beam intensity ripples that arise from diffraction and/or non-linear effects. The optical cavities combine the features of multiple passes, spatial filtering and optical reimaging and allow sufficient time for laser gain recovery.

  4. Asymmetries in the momentum distributions of electrons stripped by a XUV chirped pulse in the presence of a laser field.

    PubMed

    Bonanno, G; Bivona, S; Burlon, R; Leone, C

    2012-09-24

    The ionization of hydrogen by a chirped XUV pulse in the presence of a few cycle infrared laser pulse has been investigated. The electron momentum distribution has been obtained by treating the interaction of the atom with the XUV radiation at the first order of the time-dependent perturbation theory and describing the emitted electron through the Coulomb-Volkov wavefunction. The results of the calculations agree with the ones found by solving numerically the time-dependent Schrödinger equation. It has been found that depending on the delay between the pulses the combined effect of the XUV chirp and of the steering action on the infrared field brings about asymmetries in the electron momentum distribution. These asymmetries may give information on both the chirp and the XUV pulse duration.

  5. Nonsequential double ionization with mid-infrared laser fields

    PubMed Central

    Li, Ying-Bin; Wang, Xu; Yu, Ben-Hai; Tang, Qing-Bin; Wang, Guang-Hou; Wan, Jian-Guo

    2016-01-01

    Using a full-dimensional Monte Carlo classical ensemble method, we present a theoretical study of atomic nonsequential double ionization (NSDI) with mid-infrared laser fields, and compare with results from near-infrared laser fields. Unlike single-electron strong-field processes, double ionization shows complex and unexpected interplays between the returning electron and its parent ion core. As a result of these interplays, NSDI for mid-IR fields is dominated by second-returning electron trajectories, instead of first-returning trajectories for near-IR fields. Some complex NSDI channels commonly happen with near-IR fields, such as the recollision-excitation-with-subsequent-ionization (RESI) channel, are virtually shut down by mid-IR fields. Besides, the final energies of the two electrons can be extremely unequal, leading to novel e-e momentum correlation spectra that can be measured experimentally. PMID:27857182

  6. Nonsequential double ionization with mid-infrared laser fields

    NASA Astrophysics Data System (ADS)

    Li, Ying-Bin; Wang, Xu; Yu, Ben-Hai; Tang, Qing-Bin; Wang, Guang-Hou; Wan, Jian-Guo

    2016-11-01

    Using a full-dimensional Monte Carlo classical ensemble method, we present a theoretical study of atomic nonsequential double ionization (NSDI) with mid-infrared laser fields, and compare with results from near-infrared laser fields. Unlike single-electron strong-field processes, double ionization shows complex and unexpected interplays between the returning electron and its parent ion core. As a result of these interplays, NSDI for mid-IR fields is dominated by second-returning electron trajectories, instead of first-returning trajectories for near-IR fields. Some complex NSDI channels commonly happen with near-IR fields, such as the recollision-excitation-with-subsequent-ionization (RESI) channel, are virtually shut down by mid-IR fields. Besides, the final energies of the two electrons can be extremely unequal, leading to novel e-e momentum correlation spectra that can be measured experimentally.

  7. Field experiment of laser energy transmission and laser to electric conversion

    SciTech Connect

    Yugami, H.; Kanamori, Y.; Arashi, H.; Niino, M.; Moro, A.; Eguchi, K.; Okada, Y.; Endo, A.

    1997-12-31

    In this paper, the authors report the result of the field experiment of laser power transmission over 500m using different laser systems, i.e., CO{sub 2}, YAG, etc. The efficiency of energy transmission for long time period under various meteorological conditions was measured. They have observed large and long time scale fluctuation of beam pointing. It is found that the position of laser beam at the receiving site is correlated with the temperature difference between laser path height and ground. The laser to electricity conversion experiment has been performed using GaAs, c-Si, tandem-type a-Si, and CuInSe{sub 2} (CIS) solar cells. Finally, they briefly introduce the proposal on the space experiment of laser power transmission at Japanese Experiment Module (JEM) on the international space station.

  8. Carrier-envelope phase measurement using plasmonic-field-enhanced high-order harmonic generation of H atom in few-cycle laser pulses

    NASA Astrophysics Data System (ADS)

    Wei, Li; Guo-Li, Wang; Xiao-Xin, Zhou

    2016-05-01

    We investigate the plasmonic-field-enhanced high-order harmonic generation (HHG) of H atom driven by few-cycle laser pulses, by solving the time-dependent Schrödinger equation (TDSE). Compared with the homogeneous field, HHG spectra generated by inhomogeneous field exhibit two-plateau structure. We analyze the origin of the two plateaus by using the semiclassical trajectory method. Our results from both classical and TDSE simulations show that the cutoffs of the two plateaus are dramatically affected by the carrier-envelope phase (CEP) of laser pulse in the inhomogeneous field, even for a little longer pulse. Thus, we can determine the CEP of driving laser based on the cutoff position of HHG generated in the inhomogeneous field. Project supported by the National Natural Science Foundation of China (Grant Nos. 11264036, 11364038, and 11465016).

  9. Exploration of the electron multiple recollision dynamics in intense laser fields with Bohmian trajectories

    NASA Astrophysics Data System (ADS)

    Jooya, Hossein Z.; Telnov, Dmitry A.; Chu, Shih-I.

    2016-06-01

    Electron multiple recollision dynamics under intense midinfrared laser fields is studied by means of the de Broglie-Bohm framework of Bohmian mechanics. Bohmian trajectories contain all the information embedded in the time-dependent wave function. This makes the method suitable to investigate the coherent dynamic processes for which the phase information is crucial. In this study, the appearance of the subpeaks in the high-harmonic-generation time-frequency profiles and the asymmetric fine structures in the above-threshold ionization spectrum are analyzed by the comprehensive and intuitive picture provided by Bohmian mechanics. The time evolution of the individual electron trajectories is closely studied to address some of the major structural features of the photoelectron angular distributions.

  10. Field Evaluation of Laser Protective Eyewear

    DTIC Science & Technology

    1990-01-10

    Protective Spectacles (B-LPS), consists of a toroidal polycarbon- ate eyewrap designed to provide protection against the impact of small projectiles. Issued...environment. Another advantage of the new case is that it provides better protection against accidental crushing or impact damage when the spectacles are...block number) " A group of seventy soldiers at the National Training Center were issued Ballistic and Laser Protective Spectacles (B-LPS). The soldiers

  11. Fragmentation of negative ions in a strong laser field

    NASA Astrophysics Data System (ADS)

    Berry, Ben; Jochim, Bethany; Severt, T.; Feizollah, Peyman; Rajput, Jyoti; Hayes, D.; Carnes, K. D.; Esry, B. D.; Ben-Itzhak, I.

    2016-05-01

    The fragmentation of negative ions in a strong laser field can provide a testing ground for a variety of unique phenomena. For example, anions with a loosely bound electron allow for the study of rescattering phenomena at lower laser intensities than for neutral targets. We study the behavior of keV anion beams in an ultrafast, intense laser field. The use of a fast-beam target facilitates the measurement of neutral fragments. This capability allows us to explore laser-induced dynamics in both ionic and neutral charge states. Using a coincidence 3D momentum imaging technique, we obtain the full 3D momentum of all nuclear fragments. In this preliminary work, we study atomic (H-) and molecular (H2-,F2-)systems with the goal of identifying and controlling their fragmentation pathways. This work was supported by the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy.

  12. Electron acceleration by laser fields in a gas

    NASA Astrophysics Data System (ADS)

    Fontana, J. R.

    1991-09-01

    The strong fields lasers can produce allow high energy acceleration of charged particles. As the phase velocity of the fields cannot be matched in vacuum to the particle velocity, cumulative interaction over arbitrarily long straight trajectories is impossible. However, over limited regions a large energy gain as well as considerable focusing action can be achieved with suitably shaped laser beams. Away from boundaries, all laser fields consist of superpositions of plane wave components. We describe the properties of several practical configurations, beginning with a single plane wave. Only straight particle trajectories are considered in this analysis and it is assumed the energy is large enough so their speed is nearly constant and very close to that of light. The particles considered are electrons. The physical limitation of the interaction region may be obtained by reflecting surfaces which generate no evanescent waves, with the electron beam crossing the boundaries through holes small enough not to disturb the fields. The laser power density over these reflectors could impose a practical limit to field intensity in the interaction region. An alternative way to limit the interaction range is by bending magnets to deflect the electrons; but the energy radiated must then be taken into consideration. In the rest of this paper, no further discussion is given of interaction region boundaries, although they must be present in every case. This paper contains a quantitative analysis of the acceleration and focusing properties of a particular laser configuration, and discusses means of extending the useful interaction range by phase compensation surfaces.

  13. Ab initio non-Born-Oppenheimer simulations of rescattering dissociation of H2 in strong infrared laser fields

    NASA Astrophysics Data System (ADS)

    Li, Zhi-Chao; He, Feng

    2014-11-01

    We simulate the time-dependent Schrödinger equation and observe the rescattering dissociation of H2 in strong infrared laser fields. Two dissociation pathways are identified, i.e., the dissociation of H2+ in the 2 p σu state and the dissociation of H2 in doubly excited states. The former accounts for larger proportions as the rescattering energy is larger. The kinetic energy release of dissociative fragments reflects the temporal internuclear distance at the moment the rescattering happens.

  14. Electron and Ion Emission from Clusters exposed to Strong Laser Fields

    NASA Astrophysics Data System (ADS)

    Tiggesbämker, Josef

    2006-03-01

    When clusters interact with intense optical laser pulses energetic and highly charged atomic fragment ions e.g. are generated^1. In contrast to atoms the efficiency of the process could be enhanced by choosing a pair of optical delayed pulses instead of a single but more intense femtosecond pulse^2. In metals the stronger charging of the clusters can qualitatively be explained by a plasmon enhanced ionization process. We extended our studies and have made a compared analysis of the emission of highly charged ions and energetic electrons the interaction dynamics of intense femtosecond laser fields with nanometer-sized silver clusters. Using a pair of laser pulses with variable optical delay the time-dependent cluster response is resolved. A dramatic increase both in the atomic charge state of the ions and the maximum electron kinetic energy is observed for a certain delay of the pulses. Corresponding Vlasov calculations on a metal cluster model system indicate that enhanced cluster ionization as well as the generation of fast electrons coincide with resonant plasmon excitation.^3 *L. Köller, M. Schumacher, J. Köhn, S. Teuber, J. Tiggesbäumker, and K.-H. Meiwes-Broer, Phys. Rev. Lett. 82, 3783 (1999). *T. Döppner, Th. Fennel, Th. Diederich, J. Tiggesb äumker, and K.-H. Meiwes-Broer, Phys. Rev. Lett. 94, 013401 (2005). *Th. Fennel, G.F. Bertsch, and K.-H. Meiwes-Broer, Eur. Phys. J. D 29, 367 (2004).

  15. Attosecond Electron Wave Packet Dynamics in Strong Laser Fields

    SciTech Connect

    Johnsson, P.; Remetter, T.; Varju, K.; L'Huillier, A.; Lopez-Martens, R.; Valentin, C.; Balcou, Ph.; Kazamias, S.; Mauritsson, J.; Gaarde, M. B.; Schafer, K. J.; Mairesse, Y.; Wabnitz, H.; Salieres, P.

    2005-07-01

    We use a train of sub-200 attosecond extreme ultraviolet (XUV) pulses with energies just above the ionization threshold in argon to create a train of temporally localized electron wave packets. We study the energy transfer from a strong infrared (IR) laser field to the ionized electrons as a function of the delay between the XUV and IR fields. When the wave packets are born at the zero crossings of the IR field, a significant amount of energy ({approx}20 eV) is transferred from the field to the electrons. This results in dramatically enhanced above-threshold ionization in conditions where the IR field alone does not induce any significant ionization. Because both the energy and duration of the wave packets can be varied independently of the IR laser, they are valuable tools for studying and controlling strong-field processes.

  16. Tunable Time-Dependent Colloidal Interactions

    NASA Astrophysics Data System (ADS)

    Bergman, Andrew M.; Rogers, W. Benjamin; Manoharan, Vinothan N.

    Self-assembly of colloidal particles can be driven by changes in temperature, density, or the concentration of solutes, and it is even possible to program the thermal response and equilibrium phase transitions of such systems. It is still difficult, however, to tune how the self-assembly process varies in time. We demonstrate control over the time-dependence of colloidal interactions, using DNA-functionalized colloidal particles with binding energies that are set by the concentration of a free linker strand in solution. We control the rate at which this free strand is consumed using a catalytic DNA reaction, whose rate is governed by the concentration of a catalyst strand. Varying the concentration of the linker, its competitor, and the catalyst at a fixed temperature, we can tune the rate and degree of the formation of colloidal aggregates and their following disassembly. Close to the colloidal melting point, the timescales of these out-of-equilibrium assembly and disassembly processes are determined by the rate of the catalytic reaction. Far below the colloidal melting point, however, the effects from varying our linker and competitor concentrations dominate.

  17. Time dependent particle emission from fission products

    SciTech Connect

    Holloway, Shannon T; Kawano, Toshihiko; Moller, Peter

    2010-01-01

    Decay heating following nuclear fission is an important factor in the design of nuclear facilities; impacting a variety of aspects ranging from cooling requirements to shielding design. Calculations of decay heat, often assumed to be a simple product of activity and average decay product energy, are complicated by the so called 'pandemonium effect'. Elucidated in the 1970's this complication arises from beta-decays feeding high-energy nuclear levels; redistributing the available energy between betas and gammas. Increased interest in improving the theoretical predictions of decay probabilities has been, in part, motivated by the recent experimental effort utilizing the Total Absorption Gamma-ray Spectrometer (TAGS) to determine individual beta-decay transition probabilities to individual nuclear levels. Accurate predictions of decay heating require a detailed understanding of these transition probabilities, accurate representation of particle decays as well as reliable predictions of temporal inventories from fissioning systems. We will discuss a recent LANL effort to provide a time dependent study of particle emission from fission products through a combination of Quasiparticle Random Phase Approximation (QRPA) predictions of beta-decay probabilities, statistical Hauser-Feshbach techniques to obtain particle and gamma-ray emissions in statistical Hauser-Feshbach and the nuclear inventory code, CINDER.

  18. Generalized Sturmians in the time-dependent frame: effect of a fullerene confining potential

    NASA Astrophysics Data System (ADS)

    Frapiccini, Ana Laura; Gasaneo, Gustavo; Mitnik, Dario M.

    2017-02-01

    In this work we present a novel implementation of the Generalized Sturmian Functions in the time-dependent frame to numerically solve the time-dependent Schrödinger equation. We study the effect of the confinement of H atom in a fullerene cage for the 1s → 2p resonant transition of the atom interacting with a finite laser pulse, calculating the population of bound states and spectral density.

  19. The time-dependent Aharonov-Casher effect

    NASA Astrophysics Data System (ADS)

    Singleton, Douglas; Ulbricht, Jaryd

    2016-02-01

    In this paper we give a covariant expression for Aharonov-Casher phase. This expression is a combination of the canonical electric field, Aharonov-Casher phase plus a magnetic field phase shift. We use this covariant expression for the Aharonov-Casher phase to investigate the case of a neutral particle with a non-zero magnetic moment moving in the time dependent electric and magnetic fields of a plane electromagnetic wave background. We focus on the case where the magnetic moment of the particle is oriented so that both the electric and magnetic fields lead to non-zero phases, and we look at the interplay between these electric and magnetic phases.

  20. Observation of Broadband Time-Dependent Rabi Shifting in Microplasmas

    SciTech Connect

    Compton, Ryan; Filin, Alex; Romanov, Dmitri A.; Levis, Robert J.

    2009-11-13

    Coherent broadband radiation in the form of Rabi sidebands is observed when a ps probe laser propagates through a weakly ionized, electronically excited microplasma generated in the focus of an intense pump beam. The sidebands arise from the interaction of the probe beam with pairs of excited states of a constituent neutral atom via the probe-induced Rabi oscillation. Sideband shifting of >90 meV from the probe carrier frequency results in an effective bandwidth of 200 meV. The sidebands are controlled by the intensity and temporal profile of the probe pulse; with amplitude and shift in agreement with the predictions of a time-dependent generalized Rabi cycling model.

  1. Interaction between O{sub 2} and ZnO films probed by time-dependent second-harmonic generation

    SciTech Connect

    Andersen, S. V.; Vandalon, V.; Bosch, R. H. E. C.; Loo, B. W. H. van de; Kessels, W. M. M.; Pedersen, K.

    2014-02-03

    The interaction between O{sub 2} and ZnO thin films prepared by atomic layer deposition has been investigated by time-dependent second-harmonic generation, by probing the electric field induced by adsorbed oxygen molecules on the surface. The second-harmonic generated signal decays upon laser exposure due to two-photon assisted desorption of O{sub 2}. Blocking and unblocking the laser beam for different time intervals reveals the adsorption rate of O{sub 2} onto ZnO. The results demonstrate that electric field induced second-harmonic generation provides a versatile non-contact probe of the adsorption kinetics of molecules on ZnO thin films.

  2. Guiding-center equations for electrons in ultraintense laser fields

    SciTech Connect

    Moore, J.E.; Fisch, N.J.

    1994-01-01

    The guiding-center equations are derived for electrons in arbitrarily intense laser fields also subject to external fields and ponderomotive forces. Exhibiting the relativistic mass increase of the oscillating electrons, a simple frame-invariant equation is shown to govern the behavior of the electrons for sufficiently weak background fields and ponderomotive forces. The parameter regime for which such a formulation is valid is made precise, and some predictions of the equation are checked by numerical simulation.

  3. Guiding-center equations for electrons in ultraintense laser fields

    NASA Astrophysics Data System (ADS)

    Moore, Joel E.; Fisch, Nathaniel J.

    1994-05-01

    The guiding-center equations are derived for electrons in arbitrarily intense laser fields also subject to external fields and ponderomotive forces. Exhibiting the relativistic mass increase of the oscillating electrons, a simple frame-invariant equation is shown to govern the behavior of the electrons for sufficiently weak background fields and ponderomotive forces. The parameter regime for which such a formulation is valid is made precise, and some predictions of the equation are checked by numerical simulation.

  4. Neutron interference in the gravitational field of a ring laser

    NASA Astrophysics Data System (ADS)

    Fischetti, Robert D.; Mallett, Ronald L.

    2015-07-01

    The neutron split-beam interferometer has proven to be particularly useful in measuring Newtonian gravitational effects such as those studied by Colella, Overhauser, and Werner (COW). The development of the ring laser has led to numerous applications in many areas of physics including a recent general relativistic prediction of frame dragging in the gravitational field produced by the electromagnetic radiation in a ring laser. This paper introduces a new general technique based on a canonical transformation of the Dirac equation for the gravitational field of a general linearized spacetime. Using this technique it is shown that there is a phase shift in the interference of two neutron beams due to the frame-dragging nature of the gravitational field of a ring laser.

  5. Mathematical analysis of the temperature field during ex-vivo and in-vivo experimental laser interstitial thermotherapy (LITT) in breast tissue models

    NASA Astrophysics Data System (ADS)

    Manns, Fabrice; Milne, Peter J.; Salas, Nelson, Jr.; Pandya, Nish; Denham, David B.; Parel, Jean-Marie A.; Robinson, David S.

    1999-06-01

    Purpose: Laser interstitial thermotherapy is a promising minimally- invasive technique for the treatment of small cancers of the breast that are currently removed surgically lumpectomy. The purpose of this work was to analyze in situ temperature fields recorded with stainless-steel thermocoupled probes during experimental laser interstitial thermo-therapy (LITT). Methods: Both a CW Nd:YAG laser system emitting 20W for 25 to 30s and a 980 nm diode laser emitting 10 to 20 W for up to 1200s delivered through a fiber-optic probe were used to create localized heating in fatty cadaver pig tissue and milk as phantoms. To quantify an artifact due to direct heating of the thermocouple probes by laser radiation, experiments were also performed in air, water and intralipid solution. The temperature field around the fiber-optic probe during laser irradiation was measured every 0.3 s or 1 s with an array of up to fifteen needle thermocoupled probes. The effect of light absorption by the thermocouples probes was quantified and the time-dependence of the temperature distribution was analyzed. Results: After removal of the thermocouple artifact, the temperature was found to vary exponentially with time with a time constant of 600 to 700 s. Conclusions:The time-dependence of the interstitial temperature can be modeled by exponential functions both during ex vivo and in vivo experiments.

  6. An efficient quantum jump method for coherent energy transfer dynamics in photosynthetic systems under the influence of laser fields

    NASA Astrophysics Data System (ADS)

    Ai, Qing; Fan, Yuan-Jia; Jin, Bih-Yaw; Cheng, Yuan-Chung

    2014-05-01

    We present a non-Markovian quantum jump (NMQJ) approach for simulating coherent energy transfer dynamics in molecular systems in the presence of laser fields. By combining a coherent modified Redfield theory (CMRT) and a NMQJ method, this new approach inherits the broad-range validity from the CMRT and highly efficient propagation from the NMQJ. To implement NMQJ propagation of CMRT, we show that the CMRT master equation can be cast into a generalized Lindblad form. Moreover, we extend the NMQJ approach to treat time-dependent Hamiltonian, enabling the description of excitonic systems under coherent laser fields. As a benchmark of the validity of this new method, we show that the CMRT-NMQJ method accurately describes the energy transfer dynamics in a prototypical photosynthetic complex. Finally, we apply this new approach to simulate the quantum dynamics of a dimer system coherently excited to coupled single-excitation states under the influence of laser fields, which allows us to investigate the interplay between the photoexcitation process and ultrafast energy transfer dynamics in the system. We demonstrate that laser-field parameters significantly affect coherence dynamics of photoexcitations in excitonic systems, which indicates that the photoexcitation process must be explicitly considered in order to properly describe photon-induced dynamics in photosynthetic systems. This work should provide a valuable tool for efficient simulations of coherent control of energy flow in photosynthetic systems and artificial optoelectronic materials.

  7. Time dependence of Hawking radiation entropy

    SciTech Connect

    Page, Don N.

    2013-09-01

    If a black hole starts in a pure quantum state and evaporates completely by a unitary process, the von Neumann entropy of the Hawking radiation initially increases and then decreases back to zero when the black hole has disappeared. Here numerical results are given for an approximation to the time dependence of the radiation entropy under an assumption of fast scrambling, for large nonrotating black holes that emit essentially only photons and gravitons. The maximum of the von Neumann entropy then occurs after about 53.81% of the evaporation time, when the black hole has lost about 40.25% of its original Bekenstein-Hawking (BH) entropy (an upper bound for its von Neumann entropy) and then has a BH entropy that equals the entropy in the radiation, which is about 59.75% of the original BH entropy 4πM{sub 0}{sup 2}, or about 7.509M{sub 0}{sup 2} ≈ 6.268 × 10{sup 76}(M{sub 0}/M{sub s}un){sup 2}, using my 1976 calculations that the photon and graviton emission process into empty space gives about 1.4847 times the BH entropy loss of the black hole. Results are also given for black holes in initially impure states. If the black hole starts in a maximally mixed state, the von Neumann entropy of the Hawking radiation increases from zero up to a maximum of about 119.51% of the original BH entropy, or about 15.018M{sub 0}{sup 2} ≈ 1.254 × 10{sup 77}(M{sub 0}/M{sub s}un){sup 2}, and then decreases back down to 4πM{sub 0}{sup 2} = 1.049 × 10{sup 77}(M{sub 0}/M{sub s}un){sup 2}.

  8. Time dependence of Hawking radiation entropy

    NASA Astrophysics Data System (ADS)

    Page, Don N.

    2013-09-01

    If a black hole starts in a pure quantum state and evaporates completely by a unitary process, the von Neumann entropy of the Hawking radiation initially increases and then decreases back to zero when the black hole has disappeared. Here numerical results are given for an approximation to the time dependence of the radiation entropy under an assumption of fast scrambling, for large nonrotating black holes that emit essentially only photons and gravitons. The maximum of the von Neumann entropy then occurs after about 53.81% of the evaporation time, when the black hole has lost about 40.25% of its original Bekenstein-Hawking (BH) entropy (an upper bound for its von Neumann entropy) and then has a BH entropy that equals the entropy in the radiation, which is about 59.75% of the original BH entropy 4πM02, or about 7.509M02 ≈ 6.268 × 1076(M0/Msolar)2, using my 1976 calculations that the photon and graviton emission process into empty space gives about 1.4847 times the BH entropy loss of the black hole. Results are also given for black holes in initially impure states. If the black hole starts in a maximally mixed state, the von Neumann entropy of the Hawking radiation increases from zero up to a maximum of about 119.51% of the original BH entropy, or about 15.018M02 ≈ 1.254 × 1077(M0/Msolar)2, and then decreases back down to 4πM02 = 1.049 × 1077(M0/Msolar)2.

  9. Time Dependent Hartree Fock Equation: Gateway to Nonequilibrium Plasmas

    SciTech Connect

    James W. Dufty

    2007-04-28

    This is the Final Technical Report for DE-FG02-2ER54677 award “Time Dependent Hartree Fock Equation - Gateway to Nonequilibrium Plasmas”. Research has focused on the nonequilibrium dynamics of electrons in the presence of ions, both via basic quantum theory and via semi-classical molecular dynamics (MD) simulation. In addition, fundamental notions of dissipative dynamics have been explored for models of grains and dust, and for scalar fields (temperature) in turbulent edge plasmas. The specific topics addressed were Quantum Kinetic Theory for Metallic Clusters, Semi-classical MD Simulation of Plasmas , and Effects of Dissipative Dynamics.

  10. Time-dependent Kohn-Sham approach to quantum electrodynamics

    SciTech Connect

    Ruggenthaler, M.; Mackenroth, F.; Bauer, D.

    2011-10-15

    We prove a generalization of the van Leeuwen theorem toward quantum electrodynamics, providing the formal foundations of a time-dependent Kohn-Sham construction for coupled quantized matter and electromagnetic fields. We circumvent the symmetry-causality problems associated with the action-functional approach to Kohn-Sham systems. We show that the effective external four-potential and four-current of the Kohn-Sham system are uniquely defined and that the effective four-current takes a very simple form. Further we rederive the Runge-Gross theorem for quantum electrodynamics.

  11. Mott scattering of polarized electrons in a strong laser field

    SciTech Connect

    Manaut, B.; Taj, S.; Attaourti, Y.

    2005-04-01

    We present analytical and numerical results of the relativistic calculation of the transition matrix element S{sub fi} and differential cross sections for Mott scattering of initially polarized Dirac particles (electrons) in the presence of a strong laser field with linear polarization. We use exact Dirac-Volkov wave functions to describe the dressed electrons and the collision process is treated in the first Born approximation. The influence of the laser field on the degree of polarization of the scattered electron is reported.

  12. Measurements of laser-induced plasma temperature field in deep penetration laser welding

    NASA Astrophysics Data System (ADS)

    Chen, Genyu; Zhang, Mingjun; Zhao, Zhi; Zhang, Yi; Li, Shichun

    2013-02-01

    Laser-induced plasma in deep penetration laser welding is located inside or outside the keyhole, namely, keyhole plasma or plasma plume, respectively. The emergence of laser-induced plasma in laser welding reveals important information of the welding technological process. Generally, electron temperature and electron density are two important characteristic parameters of plasma. In this paper, spectroscopic measurements of electron temperature and electron density of the keyhole plasma and plasma plume in deep penetration laser welding conditions were carried out. To receive spectra from several points separately and simultaneously, an Optical Multi-channel Analyser (OMA) was developed. On the assumption that the plasma was in local thermal equilibrium, the temperature was calculated with the spectral relative intensity method. The spectra collected were processed with Abel inversion method to obtain the temperature fields of keyhole plasma and plasma plume.

  13. Multifunctional quantum node based on double quantum dot in laser and cavity fields

    NASA Astrophysics Data System (ADS)

    Tsukanov, Alexander V.

    2016-12-01

    The concept of multifunctional device (a quantum node) composed of a semiconductor single-electron four-level doublequantum dot coupled to an optical microcavity resonator is developed. The terahertz laser field and voltage biases provide an external control. The structure enables flexible driving via appropriate variations of field amplitudes and switching between resonant and off-resonant modes. As shown this hybrid electron-photon system can be used as the charge qubit with flying-to-stationary qubit conversion or the single-photon transistor and several others. Each of listed devices works in the specific regime of system evolution. For example, the qubit is robust when the optical resonator and laser Rabi frequencies dominate the dissipation rates - the so-called strong coupling or coherent regime. From another hand, in order to attain the steady-state one has to work in the so-called weak coupling or incoherent regime when the dissipation rates are comparable to or greater than the Rabi frequencies. Further, the single-photon driving is required for spectroscopic applications of this system. We numerically investigate the population dynamics to reveal the parameter choice corresponding to each device. The model is based on Lindblad formalism where all incoherent processes are considered as the markovian ones. The time dependencies of populations and spectrograms for different pairs of parameters are obtained. The specific features concerned with working characteristics of the quantum node in different modes are discussed.

  14. Fast electrons from electron-ion collisions in strong laser fields

    SciTech Connect

    Kull, H.-J.; Tikhonchuk, V.T.

    2005-06-15

    Electron-ion collisions in the presence of a strong laser field lead to a distribution of fast electrons with maximum energy E{sub max}=(k{sub 0}+2v{sub 0}){sup 2}/2(a.u.), where k{sub 0} is the impact and v{sub 0} the quiver velocity of the electron. The energy spectrum is calculated by two approaches: (1) The time-dependent Schroedinger equation is numerically solved for wave packet scattering from a one-dimensional softcore Coulomb potential. Multiphoton energy spectra are obtained demonstrating a separation of the energy spectrum into an exponential distribution for transmission and a plateau distribution for reflection. (2) The energy spectrum is analytically calculated in the framework of classical instantaneous Coulomb collisions with random impact parameters and random phases of the laser field. An exact solution for the energy spectrum is obtained from which the fraction of fast electrons in the plateau region can be estimated.

  15. Laser-generated magnetic fields in quasi-hohlraum geometries

    NASA Astrophysics Data System (ADS)

    Pollock, Bradley; Turnbull, David; Ross, Steven; Hazi, Andrew; Ralph, Joseph; Lepape, Sebastian; Froula, Dustin; Haberberger, Dan; Moody, John

    2014-10-01

    Laser-generated magnetic fields of 10--40 T have been produced with 100--4000 J laser drives at Omega EP and Titan. The fields are generated using the technique described by Daido et al. [Phys. Rev. Lett. 56, 846 (1986)], which works by directing a laser through a hole in one plate to strike a second plate. Hot electrons generated in the laser-produced plasma on the second plate collect on the first plate. A strap connects the two plates allowing a current of 10 s of kA to flow and generate a solenoidal magnetic field. The magnetic field is characterized using Faraday rotation, b-dot probes, and proton radiography. Further experiments to study the effect of the magnetic field on hohlraum performance are currently scheduled for Omega. This work was performed under the auspices of the United States Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA-27344.

  16. Energy equipartitioning in the classical time-dependent Hartree approximation

    NASA Astrophysics Data System (ADS)

    Straub, John E.; Karplus, Martin

    1991-05-01

    In the classical time-dependent Hartree approximation (TDH), the dynamics of a single molecule is approximated by that of a ``field'' (each field being N ``copies'' of the molecule which are transparent to one another while interacting with the system via a scaled force). It is shown that when some molecules are represented by a field of copies, while other molecules are represented normally, the average kinetic energy of the system increases linearly with the number of copies and diverges in the limit of large N. Nevertheless, the TDH method with appropriate energy scaling can serve as a useful means of enhancing the configurational sampling for problems involving coupled systems with disparate numbers of degrees of freedom.

  17. Mean-field dynamics of a Bose-Einstein condensate in a time-dependent triple-well trap: Nonlinear eigenstates, Landau-Zener models, and stimulated Raman adiabatic passage

    SciTech Connect

    Graefe, E. M.; Korsch, H. J.; Witthaut, D.

    2006-01-15

    We investigate the dynamics of a Bose-Einstein condensate in a triple-well trap in a three-level approximation. The interatomic interactions are taken into account in a mean-field approximation (Gross-Pitaevskii equation), leading to a nonlinear three-level model. Additional eigenstates emerge due to the nonlinearity, depending on the system parameters. Adiabaticity breaks down if such a nonlinear eigenstate disappears when the parameters are varied. The dynamical implications of this loss of adiabaticity are analyzed for two important special cases: A three-level Landau-Zener model and the stimulated Raman adiabatic passage (STIRAP) scheme. We discuss the emergence of looped levels for an equal-slope Landau-Zener model. The Zener tunneling probability does not tend to zero in the adiabatic limit and shows pronounced oscillations as a function of the velocity of the parameter variation. Furthermore we generalize the STIRAP scheme for adiabatic coherent population transfer between atomic states to the nonlinear case. It is shown that STIRAP breaks down if the nonlinearity exceeds the detuning.

  18. Time-Dependent Rate Phenomenon in Viruses

    PubMed Central

    Aiewsakun, Pakorn

    2016-01-01

    ABSTRACT Among the most fundamental questions in viral evolutionary biology are how fast viruses evolve and how evolutionary rates differ among viruses and fluctuate through time. Traditionally, viruses are loosely classed into two groups: slow-evolving DNA viruses and fast-evolving RNA viruses. As viral evolutionary rate estimates become more available, it appears that the rates are negatively correlated with the measurement timescales and that the boundary between the rates of DNA and RNA viruses might not be as clear as previously thought. In this study, we collected 396 viral evolutionary rate estimates across almost all viral genome types and replication strategies, and we examined their rate dynamics. We showed that the time-dependent rate phenomenon exists across multiple levels of viral taxonomy, from the Baltimore classification viral groups to genera. We also showed that, by taking the rate decay dynamics into account, a clear division between the rates of DNA and RNA viruses as well as reverse-transcribing viruses could be recovered. Surprisingly, despite large differences in their biology, our analyses suggested that the rate decay speed is independent of viral types and thus might be useful for better estimation of the evolutionary time scale of any virus. To illustrate this, we used our model to reestimate the evolutionary timescales of extant lentiviruses, which were previously suggested to be very young by standard phylogenetic analyses. Our analyses suggested that these viruses are millions of years old, in agreement with paleovirological evidence, and therefore, for the first time, reconciled molecular analyses of ancient and extant viruses. IMPORTANCE This work provides direct evidence that viral evolutionary rate estimates decay with their measurement timescales and that the rate decay speeds do not differ significantly among viruses despite the vast differences in their molecular features. After adjustment for the rate decay dynamics, the

  19. A time-dependent variational principle and the time-dependent Hartree approximation in hydrodynamical form

    NASA Astrophysics Data System (ADS)

    Lill, J. V.; Haftel, M. I.; Herling, G. H.

    1989-05-01

    A quantum mechanical time-dependent variational principle is generalized using the classical theory of fluids to obtain a variational principle suitable for the fluid dynamical description of mixed state quantum mechanics. A newly derived set of moment equations, in both standard and renormalized form, can be derived with the aid of this principle through minimization of the error in expressing the total derivative of the Wigner function. Coupled systems are studied in the time-dependent Hartree (TDH) approximation using a novel variational principle, and the renormalization procedure used earlier in the examination of single particle dynamics is extended to the TDH analysis. Use of a local Maxwellian ansatz for each particle results in a particularly simple ``two-fluid'' theory, the TDH/LM approximation, which does not violate the standard and renormalized energy conservation theorems derived earlier for the single particle equations. The fluid dynamical TDH/LM approximation is shown to possess a simple semiclassical interpretation.

  20. Electron emission and fragmentation of molecules in intense laser fields

    NASA Astrophysics Data System (ADS)

    Ueda, K.; Prümper, G.; Hatamoto, T.; Okunishi, M.; Mathur, D.

    2007-06-01

    We have constructed an apparatus for high-resolution electron spectroscopy and electron-ion coincidence experiments on gas-phase molecules in intense laser fields. The apparatus comprises an electron time-of-flight (TOF) spectrometer and an ion TOF spectrometer with a position detector, placed on either side of an effusive molecular beam. The ionizing radiation is either the fundamental (800 nm wavelength) of a Ti:sapphire laser or frequency doubled 400-nm light, with pulse durations of ~ 150 fs and the repetition rate of 1 kHz. We have investigated the electron emission and fragmentation of linear alcohol molecules, methanol, ethanol and 1-propanol, in laser fields with peak intensities up to ~ 1×10 14 W/cm2. Details of our apparatus are described along with an overview of some recent results.

  1. Theory of a ring laser. [electromagnetic field and wave equations

    NASA Technical Reports Server (NTRS)

    Menegozzi, L. N.; Lamb, W. E., Jr.

    1973-01-01

    Development of a systematic formulation of the theory of a ring laser which is based on first principles and uses a well-known model for laser operation. A simple physical derivation of the electromagnetic field equations for a noninertial reference frame in uniform rotation is presented, and an attempt is made to clarify the nature of the Fox-Li modes for an open polygonal resonator. The polarization of the active medium is obtained by using a Fourier-series method which permits the formulation of a strong-signal theory, and solutions are given in terms of continued fractions. It is shown that when such a continued fraction is expanded to third order in the fields, the familiar small-signal ring-laser theory is obtained.

  2. Effect of intense laser IR fields on triatomic molecules

    NASA Astrophysics Data System (ADS)

    Ivanov, S. V.; Panchenko, V. Ia.; Chugunov, A. V.

    1986-04-01

    Theoretical and experimental results on the effect of intense laser IR fields on triatomic molecular gases are presented with particular emphasis on ozone. Experiments were conducted in single- and double-frequency IR fields at power densities ranging from 10 to the -6th to 10 GW/sq cm in the pulsed regime and 0.001 to 100 W/sq cm in the CW regime; studies were performed using a TEA CO2 laser system. Attention is given to: the nonlinear absorption spectrum; the dependence of absorption in ozone on the power density of incident radiation; results of numerical solutions; the analytical solution; two-photon resonances in the ozone absorption spectrum; the spectrum of double-frequency IR-IR absorption; cascade-excitation channels; and laser-stimulated explosion in ozone.

  3. Temperature field around a laser-heated coal particle

    SciTech Connect

    Feng, B.; Liu, Y.H.; Zhou, Y.B.; Liu, Z.H.; Zheng, C.G.

    1997-12-31

    Holography was used to measure the temperature field around a laser heated coal particle. A man-made coal particle (with the size of 5mm in diameter and 5mm in length) was ignited by a laser beam (with the maximum power of 15W). And then the temperature distribution around the particle was obtained from the holograph which was developed by the authors. A bituminous coal, an anthracite and a sub-bituminous coal were used. It was interesting to find that there exists a zone near the particle surface where the temperature is higher than that at the surface for the bituminous coal during the combustion of the coal although the phenomenon was not found for the other coals. A mathematical model taking into account the laser induced energy was developed to calculate the temperature field around the particle. The predicted results were compared with the experimental ones.

  4. Collimation of laser-produced plasmas using axial magnetic field

    SciTech Connect

    Roy, Amitava; Harilal, Sivanandan S.; Hassan, Syed M.; Endo, Akira; Mocek, Tomas; Hassanein, A.

    2015-06-01

    We investigated the expansion dynamics of laser-produced plasmas expanding into an axial magnetic field. Plasmas were generated by focusing 1.064 µm Nd:YAG laser pulses onto a planar tin target in vacuum and allowed to expand into a 0.5 T magnetic-filed where field lines were aligned along the plume expansion direction. Gated images employing intensified CCD showed focusing of the plasma plume, which were also compared with results obtained using particle-in-cell modelling methods. The estimated density and temperature of the plasma plumes employing emission spectroscopy revealed significant changes in the presence and absence of the 0.5T magnetic field. In the presence of the field, the electron temperature is increased with distance from the target, while the density showed opposite effects.

  5. Time-dependent Models of Magnetospheric Accretion onto Young Stars

    NASA Astrophysics Data System (ADS)

    Robinson, C. E.; Owen, J. E.; Espaillat, C. C.; Adams, F. C.

    2017-04-01

    Accretion onto Classical T Tauri stars is thought to take place through the action of magnetospheric processes, with gas in the inner disk being channeled onto the star’s surface by the stellar magnetic field lines. Young stars are known to accrete material in a time-variable manner, and the source of this variability remains an open problem, particularly on the shortest (∼day) timescales. Using one-dimensional time-dependent numerical simulations that follow the field line geometry, we find that for plausibly realistic young stars, steady-state transonic accretion occurs naturally in the absence of any other source of variability. However, we show that if the density in the inner disk varies smoothly in time with ∼day-long timescales (e.g., due to turbulence), this complication can lead to the development of shocks in the accretion column. These shocks propagate along the accretion column and ultimately hit the star, leading to rapid, large amplitude changes in the accretion rate. We argue that when these shocks hit the star, the observed time dependence will be a rapid increase in accretion luminosity, followed by a slower decline, and could be an explanation for some of the short-period variability observed in accreting young stars. Our one-dimensional approach bridges previous analytic work to more complicated multi-dimensional simulations and observations.

  6. Time-dependent deformations on marine clays on submarine slopes

    SciTech Connect

    Silva, A.J.; Brandes, H.; Sadd, M.H.; Tian, W.M. )

    1990-06-01

    Evidence from geological and geophysical records indicates that time-dependent deformations occur on or within many submarine slopes. Laboratory studies on marine clays from the slope/rise and the ocean's basin have shown that these clays are generally quite viscous and therefore can be expected to deform in the field even under such small stresses as those caused by the downslope component of gravity on relatively gentle slopes. The nature and extent of these deformations has important geologic and engineering applications and depends on a number of factors. A research program at the University of Rhode Island is under way to study these factors, make predictions on rates of displacement, and identify environmental conditions that may lead to catastrophic mass failures. A laboratory testing program on the time-dependent characteristics of marine clays has been under way for a number of years. The data include, among others, long-term drained triaxial, one-dimensional, and direct simple shear creep tests. These results along with practical considerations are used to select a constitutive model for inclusion in the numerical code. Sediment deposits encountered on the continental slope and rise can vary substantially both in composition and behavior over relatively short distances. To analyze the integrated behavior of such a continuum, the authors have selected the finite element method. The code being developed will initially include a numerical model proposed by other investigators. With the aid of the developed methodology, creep deformations can be studied for a number of field cases of interest.

  7. Quantum control of electron wave packet during high harmonic process of H2(+) in a combination of a circularly polarized laser field and a Terahertz field.

    PubMed

    Ge, Xin-Lei; Du, Hui; Guo, Jing; Liu, Xue-Shen

    2015-04-06

    By solving a two-dimensional time-dependent Schrödinger equation we investigate high harmonic generation (HHG) and isolated attosecond pulse generation for the H2+ molecular ion in a circularly polarized laser pulse combined with a Terahertz (THz) field. The harmonic intensity can be greatly enhanced and a continuum spectrum can be obtained when a THz field is added. The HHG process is studied by the semi-classical three-step model and the time-frequency analysis. Our studies show that only short trajectories contribute to HHG. Furthermore, we present the temporal evolution of the probability density of electron wave packet, which perfectly shows a clear picture of the electron's two-time recombination when a THz field is added, and it is the main mechanism of HHG. By superposing the harmonics in the range of 216-249 eV, an isolated attosecond pulse with a duration of about 69 attoseconds can be generated.

  8. Atomic Beam Laser Spectrometer for In-field Isotopic Analysis

    SciTech Connect

    Castro, Alonso

    2016-06-22

    This is a powerpoint presentation for the DTRA quarterly program review that goes into detail about the atomic beam laser spectrometer for in-field isotopic analysis. The project goals are the following: analysis of post-detonation debris, determination of U and Pu isotopic composition, and fieldable prototype: < 2ft3, < 1000W.

  9. Low-field MRI of laser polarized noble gas

    NASA Technical Reports Server (NTRS)

    Tseng, C. H.; Wong, G. P.; Pomeroy, V. R.; Mair, R. W.; Hinton, D. P.; Hoffmann, D.; Stoner, R. E.; Hersman, F. W.; Cory, D. G.; Walsworth, R. L.

    1998-01-01

    NMR images of laser polarized 3He gas were obtained at 21 G using a simple, homebuilt instrument. At such low fields magnetic resonance imaging (MRI) of thermally polarized samples (e.g., water) is not practical. Low-field noble gas MRI has novel scientific, engineering, and medical applications. Examples include portable systems for diagnosis of lung disease, as well as imaging of voids in porous media and within metallic systems.

  10. Atomic electron correlations in intense laser fields

    SciTech Connect

    DiMauro, L.F.; Sheehy, B.; Walker, B. Agostini, P.A. Kulander, K.C.

    1999-06-01

    This talk examines two distinct cases in strong optical fields where electron correlation plays an important role in the dynamics. In the first example, strong coupling in a two-electron-like system is manifested as an intensity-dependent splitting in the ionized electron energy distribution. This two-electron phenomenon (dubbed continuum-continuum Autler-Townes effect) is analogous to a strongly coupled two-level, one-electron atom but raises some intriguing questions regarding the exact nature of electron-electron correlation. The second case examines the evidence for two-electron ionization in the strong-field tunneling limit. Although our ability to describe the one-electron dynamics has obtained a quantitative level of understanding, a description of the two (multiple) electron ionization remains unclear. {copyright} {ital 1999 American Institute of Physics.}

  11. Atomic electron correlations in intense laser fields

    SciTech Connect

    DiMauro, L.F.; Sheehy, B.; Walker, B.; Agostini, P.A.; Kulander, K.C.

    1998-11-01

    This talk examines two distinct cases in strong optical fields where electron correlation plays an important role in the dynamics. In the first example, strong coupling in a two-electron-like system is manifested as an intensity-dependent splitting in the ionized electron energy distribution. This two-electron phenomenon (dubbed continuum-continuum Autler-Townes effect) is analogous to a strongly coupled two-level, one-electron atom but raises some intriguing questions regarding the exact nature of electron-electron correlation. The second case examines the evidence for two-electron ionization in the strong-field tunneling limit. Although their ability to describe the one-electron dynamics has obtained a quantitative level of understanding, a description of the two (multiple) electron ionization remains unclear.

  12. Atomic electron correlations in intense laser fields

    SciTech Connect

    DiMauro, L. F.; Sheehy, B.; Walker, B.; Agostini, P. A.; Kulander, K. C.

    1999-06-11

    This talk examines two distinct cases in strong optical fields where electron correlation plays an important role in the dynamics. In the first example, strong coupling in a two-electron-like system is manifested as an intensity-dependent splitting in the ionized electron energy distribution. This two-electron phenomenon (dubbed continuum-continuum Autler-Townes effect) is analogous to a strongly coupled two-level, one-electron atom but raises some intriguing questions regarding the exact nature of electron-electron correlation. The second case examines the evidence for two-electron ionization in the strong-field tunneling limit. Although our ability to describe the one-electron dynamics has obtained a quantitative level of understanding, a description of the two (multiple) electron ionization remains unclear.

  13. Atomic electron correlations in intense laser fields

    SciTech Connect

    Agostini, P A; DiMauro, L F; Kulander, K; Sheehy, B; Walker, B

    1998-09-03

    Abstract. This talk examines two distinct cases in strong opbical fields where electron correlation plays an important role in the dynamic.s. In the first. example, strong coupling in a two-electron-like system is manifested as an intensity-dependent splitting in the ionized electron energy distribution. This two-electron phenomenon (dubbed continuum-continuum Autler-Townes effect) is analogous to a strongly coupled two- level, one-electron atom but raises some intriguing questions regarding the exact nature of electron-electron correlation. The second case examines the evidence for two-electron ionization in the strong-field tunneling limit. Although our ability to describe the one- electron dynamics has obtained a quantitative level of understanding, a description of the two (multiple) electron ionization remains unc

  14. Quantum optical signatures in strong-field laser physics: Infrared photon counting in high-order-harmonic generation

    NASA Astrophysics Data System (ADS)

    Gonoskov, I. A.; Tsatrafyllis, N.; Kominis, I. K.; Tzallas, P.

    2016-09-01

    We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent Schrödinger equation (TDSE). This wave function provides information about the quantum optical features of the interaction not accessible by semi-classical theories. With this approach we can reveal the quantum optical properties of high harmonic generation (HHG) process in gases by measuring the photon statistics of the transmitted infrared (IR) laser radiation. This work can lead to novel experiments in high-resolution spectroscopy in extreme-ultraviolet (XUV) and attosecond science without the need to measure the XUV light, while it can pave the way for the development of intense non-classical light sources.

  15. Quantum optical signatures in strong-field laser physics: Infrared photon counting in high-order-harmonic generation.

    PubMed

    Gonoskov, I A; Tsatrafyllis, N; Kominis, I K; Tzallas, P

    2016-09-07

    We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent Schrödinger equation (TDSE). This wave function provides information about the quantum optical features of the interaction not accessible by semi-classical theories. With this approach we can reveal the quantum optical properties of high harmonic generation (HHG) process in gases by measuring the photon statistics of the transmitted infrared (IR) laser radiation. This work can lead to novel experiments in high-resolution spectroscopy in extreme-ultraviolet (XUV) and attosecond science without the need to measure the XUV light, while it can pave the way for the development of intense non-classical light sources.

  16. Quantum optical signatures in strong-field laser physics: Infrared photon counting in high-order-harmonic generation

    PubMed Central

    Gonoskov, I. A.; Tsatrafyllis, N.; Kominis, I. K.; Tzallas, P.

    2016-01-01

    We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent Schrödinger equation (TDSE). This wave function provides information about the quantum optical features of the interaction not accessible by semi-classical theories. With this approach we can reveal the quantum optical properties of high harmonic generation (HHG) process in gases by measuring the photon statistics of the transmitted infrared (IR) laser radiation. This work can lead to novel experiments in high-resolution spectroscopy in extreme-ultraviolet (XUV) and attosecond science without the need to measure the XUV light, while it can pave the way for the development of intense non-classical light sources. PMID:27601191

  17. Semiclassical theory of unimolecular dissociation induced by a laser field

    NASA Technical Reports Server (NTRS)

    Yuan, J.-M.; George, T. F.

    1978-01-01

    A semiclassical nonperturbative theory of direct photodissociation in a laser field is developed in which photon absorption and dissociation are treated in a unified fashion. This is achieved by visualizing nuclear dynamics as a representative particle moving on electronic-field surfaces. Methods are described for calculating dissociation rates and probabilities by Monte Carlo selection of initial conditions and integration of classical trajectories on these surfaces. This unified theory reduces to the golden rule expression in the weak-field and short-time limits, and predicts nonlinear behavior, i.e., breakdown of the golden rule expression in intense fields. Field strengths above which lowest-order perturbation theory fails to work have been estimated for some systems. Useful physical insights provided by the electronic-field representation have been illustrated. Intense field effects are discussed which are amenable to experimental observation. The semiclassical methods used here are also applicable to multiple-surface dynamics in fieldfree unimolecular and bimolecular reactions.

  18. A compact field-portable double-pulse laser system to enhance laser induced breakdown spectroscopy

    NASA Astrophysics Data System (ADS)

    Li, Shuo; Liu, Lei; Yan, Aidong; Huang, Sheng; Huang, Xi; Chen, Rongzhang; Lu, Yongfeng; Chen, Kevin

    2017-02-01

    This paper reports the development of a compact double-pulse laser system to enhance laser induced breakdown spectroscopy (LIBS) for field applications. Pumped by high-power vertical-surface emitting lasers, the laser system that produces 16 ns pulse at 12 mJ/pulse with total weight less than 10 kg is developed. The inter-pulse delay can be adjusted from 0 μ s with 0.5 μ s increment. Several LIBS experiments were carried out on NIST standard aluminum alloy samples. Comparing with the single-pulse LIBS, up to 9 times enhancement in atomic emission line was achieved with continuum background emission reduced by 70%. This has led to up to 10 times improvement in the limit of detection. Signal stability was also improved by 128% indicating that a more robust and accurate LIBS measurement can be achieved using a compact double-pulse laser system. This paper presents a viable and field deployable laser tool to dramatically improve the sensitivity and applicability of LIBS for a wide array of applications.

  19. Atoms, molecules and clusters in intense laser fields

    NASA Astrophysics Data System (ADS)

    Walters, Zachary B.

    Recent advances in the technology of intense, short laser pulses have opened the possibility of investigating processes in atoms, molecules and clusters in which the normal intramolecular forces between electrons and nuclei, and between different electrons, are rivaled in strength by interactions with the driving laser, or with a cluster plasma. Experiments using rescattered electrons offer a means of probing atomic and molecular processes on ultrafast timescales. This thesis extends techniques and concepts of atomic and molecular physics to describe physics in the strong field regime. This involves investigating how electron scattering from atoms and molecules is affected by the intense and time-varying electric field of the laser, the effect of such scattering on experimental observables, and the role of intramolecular structure on strong field processes. Also investigated is the evolution of van derWaals atomic clusters when subject to intense laser pulses in the VUV regime. Here processes such as photoionization, inverse bremsstrahlung heating, and collisional ionization and recombination are affected both by the non-hydrogenic nature of the relevant atomic potentials but also by the screening of these potentials by the cluster plasma.

  20. Mathematical model of SPOC with a time dependent reactive field

    NASA Astrophysics Data System (ADS)

    Ohtaki, Masako

    2006-03-01

    In general the muscle is in one of the two state possible states, relaxation or contraction. These contractions result from relative sliding of myosin and actin in the sarcomere, which is the contraction structure unit of skeletal muscle. The switching between two states is depending on the Ca2+ concentrations. However another state has been detected between these two states. In the third state, that is SPontaneous Oscillatory Contraction (SPOC), sarcomere repeats contraction and extension spontaneously. Muscle fibers are composed of hundreds of sarcomeres in series and one sarcomea also is composed of hundreds of myosin. In microscopic, the force generated by actin and myosin interaction occurs stochastically. SPOC, however, is macroscopically observable and there are regular oscillations. To understand SPOC mechanism, we propose a model for SPOC based on chemical reaction including mechanical process.

  1. Effect of solenoidal magnetic field on drifting laser plasma

    NASA Astrophysics Data System (ADS)

    Takahashi, Kazumasa; Okamura, Masahiro; Sekine, Megumi; Cushing, Eric; Jandovitz, Peter

    2013-04-01

    An ion source for accelerators requires to provide a stable waveform with a certain pulse length appropriate to the application. The pulse length of laser ion source is easy to control because it is expected to be proportional to plasma drifting distance. However, current density decay is proportional to the cube of the drifting distance, so large current loss will occur under unconfined drift. We investigated the stability and current decay of a Nd:YAG laser generated copper plasma confined by a solenoidal field using a Faraday cup to measure the current waveform. It was found that the plasma was unstable at certain magnetic field strengths, so a baffle was introduced to limit the plasma diameter at injection and improve the stability. Magnetic field, solenoid length, and plasma diameter were varied in order to find the conditions that minimize current decay and maximize stability.

  2. Free charged particle behavior in intense laser fields

    NASA Astrophysics Data System (ADS)

    Fradkin, D. M.

    1984-03-01

    Theoretical studies were performed examining the effect of intense laser fields, together with auxiliary electromagnetic field configuration, on the behavior of otherwise free charged particles. The Lorentz-Dirac classical equation was employed to determine the effect of radiation reaction on the transfer of asymptotic energy momentum to a particle by a single intense plane wave pulse. The added effect due to a uniform magnetic field along the pulse propagation direction was determined. Single particle Dirac theory was employed to analyze particle polarization direction changes in a quantum-mechanical model. The general nature of the Lorentz transformation as a active transformation connecting initial and final states was determined, in which a single state characterization parameter was left unspecified. Analytic and computer studies were made of the effect of two simultaneous laser pulses, propagating in opposite directions on particle dynamics.

  3. Satellite laser ranging and gravity field modeling accuracy

    NASA Technical Reports Server (NTRS)

    Rosborough, George W.

    1990-01-01

    Gravitational field mismodeling procedures errors in the estimated orbital motion of near Earth satellites. This effect is studied using a linear perturbation approach following the analysis of Kaula. The perturbations in the orbital position as defined by either orbital elements or Cartesian components are determined. From these perturbations it is possible to ascertain the expected signal due to gravitational mismodeling that would be present in station-to-satellite laser ranging measurements. This expected signal has been estimated for the case of the Lageos satellite and using the predicted uncertainties of the GEM-T1 and GEM-T2 gravity field models. The results indicate that observable signal still exists in the laser range residuals given the current accuracy of the range measurements and the accuracy of the gravity field models.

  4. Transition from SAMO to Rydberg State Ionization in C60 in Femtosecond Laser Fields

    PubMed Central

    2016-01-01

    The transition between two distinct ionization mechanisms in femtosecond laser fields at 785 nm is observed for C60 molecules. The transition occurs in the investigated intensity range from 3 to 20 TW/cm2 and is visualized in electron kinetic energy spectra below the one-photon energy (1.5 eV) obtained via velocity map imaging. Assignment of several observed broad spectral peaks to ionization from superatom molecular orbitals (SAMOs) and Rydberg states is based on time-dependent density functional theory simulations. We find that ionization from SAMOs dominates the spectra for intensities below 5 TW/cm2. As the intensity increases, Rydberg state ionization exceeds the prominence of SAMOs. Using short laser pulses (20 fs) allowed uncovering of distinct six-lobe photoelectron angular distributions with kinetic energies just above the threshold (below 0.2 eV), which we interpret as over-the-barrier ionization of shallow f-Rydberg states in C60. PMID:27934203

  5. Time Circular Birefringence in Time-Dependent Magnetoelectric Media

    PubMed Central

    Zhang, Ruo-Yang; Zhai, Yan-Wang; Lin, Shi-Rong; Zhao, Qing; Wen, Weijia; Ge, Mo-Lin

    2015-01-01

    Light traveling in time-dependent media has many extraordinary properties which can be utilized to convert frequency, achieve temporal cloaking, and simulate cosmological phenomena. In this paper, we focus on time-dependent axion-type magnetoelectric (ME) media, and prove that light in these media always has two degenerate modes with opposite circular polarizations corresponding to one wave vector , and name this effect “time circular birefringence” (TCB). By interchanging the status of space and time, the pair of TCB modes can appear simultaneously via “time refraction” and “time reflection” of a linear polarized incident wave at a time interface of ME media. The superposition of the two TCB modes causes the “time Faraday effect”, namely the globally unified polarization axes rotate with time. A circularly polarized Gaussian pulse traversing a time interface is also studied. If the wave-vector spectrum of a pulse mainly concentrates in the non-traveling-wave band, the pulse will be trapped with nearly fixed center while its intensity will grow rapidly. In addition, we propose an experimental scheme of using molecular fluid with external time-varying electric and magnetic fields both parallel to the direction of light to realize these phenomena in practice. PMID:26329928

  6. High-order-harmonic generation in an elliptically polarized laser field: analytic form of the electron wave packet

    NASA Astrophysics Data System (ADS)

    Sarantseva, T. S.; Silaev, A. A.; Manakov, N. L.

    2017-04-01

    An analytic expression for the electron wave packet (EWP) describing high-order harmonic generation (HHG) by atoms in an intense laser field with small ellipticity is derived quantum mechanically in the tunneling limit within the time-dependent effective range theory. This result is valid over a wide interval of returned electron energies in the HHG plateau region and generalizes the previous result for HHG rates obtained by Frolov M V et al (2012 Phys. Rev. A 86 063406) only for the HHG plateau cutoff region. It is shown that the most important difference from the case of a linearly polarized field originates from a nonzero electron energy at the moment of ionization in an elliptically polarized field that, in turn, results in the dependence of ionization factor in the EWP on the returning electron energy. Our analytic result for the EWP averaged over interference oscillations in the HHG spectrum is applied for analysis of the laser wavelength scaling of the HHG yield induced by an elliptically polarized midinfrared laser field as well as for the improvement of the recently suggested method of elliptic HHG spectroscopy for retrieving both the energy and angular dependence of the photorecombination cross section of the target atom (see Frolov M V et al 2016 Phys. Rev. A 93 031403).

  7. Nonadiabatic tunnel ionization of current-carrying orbitals of prealigned linear molecules in strong circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Liu, Kunlong; Barth, Ingo

    2016-10-01

    We derive the analytical formula of the ratio of the ionization rates of degenerate valence π± orbitals of prealigned linear molecules in strong circularly polarized (CP) laser fields. Interestingly, our theory shows that the ionization ratio for molecular orbitals with opposite azimuthal quantum numbers ±|m | (e.g., π±) is identical to that for atomic orbitals with the same ±|m | (e.g., p±). In general, the electron counter-rotating to the CP laser field tunnels more easily, not only for atoms but also for linear molecules. Our theoretical predictions are then verified by numerically solving the three-dimensional time-dependent Schrödinger equation for the ionization of the prealigned nitric oxide (NO) molecule in strong CP laser fields. Due to the spin-orbital coupling in the electronic ground state of NO and the sensitivity of ionization to the sense of electron rotation, the ionization of NO in CP fields can produce spin-polarized photoelectrons with high controllability of spin polarization up to 100 % .

  8. Femtosecond Laser Processing by Using Patterned Vector Optical Fields

    PubMed Central

    Lou, Kai; Qian, Sheng-Xia; Ren, Zhi-Cheng; Tu, Chenghou; Li, Yongnan; Wang, Hui-Tian

    2013-01-01

    We present and demonstrate an approach for femtosecond laser processing by using patterned vector optical fields (PVOFs) composed of multiple individual vector optical fields. The PVOFs can be flexibly engineered due to the diversity of individual vector optical fields in spatial arrangement and distribution of states of polarization, and it is easily created with the aid of a spatial light modulator. The focused PVOFs will certainly result in various interference patterns, which are then used to fabricate multi-microholes with various patterns on silicon. The present approach can be expanded to fabricate three-dimensional microstructures based on two-photon polymerization. PMID:23884360

  9. Quasistatic limit of the strong-field approximation describing atoms in intense laser fields: Circular polarization

    SciTech Connect

    Bauer, Jaroslaw H.

    2011-03-15

    In the recent work of Vanne and Saenz [Phys. Rev. A 75, 063403 (2007)] the quasistatic limit of the velocity gauge strong-field approximation describing the ionization rate of atomic or molecular systems exposed to linearly polarized laser fields was derived. It was shown that in the low-frequency limit the ionization rate is proportional to the laser frequency {omega} (for a constant intensity of the laser field). In the present work I show that for circularly polarized laser fields the ionization rate is proportional to {omega}{sup 4} for H(1s) and H(2s) atoms, to {omega}{sup 6} for H(2p{sub x}) and H(2p{sub y}) atoms, and to {omega}{sup 8} for H(2p{sub z}) atoms. The analytical expressions for asymptotic ionization rates (which become nearly accurate in the limit {omega}{yields}0) contain no summations over multiphoton contributions. For very low laser frequencies (optical or infrared) these expressions usually remain with an order-of-magnitude agreement with the velocity gauge strong-field approximation.

  10. Holocinematographic velocimeter for measuring time-dependent, three-dimensional flows

    NASA Technical Reports Server (NTRS)

    Beeler, George B.; Weinstein, Leonard M.

    1987-01-01

    Two simulatneous, orthogonal-axis holographic movies are made of tracer particles in a low-speed water tunnel to determine the time-dependent, three-dimensional velocity field. This instrument is called a Holocinematographic Velocimeter (HCV). The holographic movies are reduced to the velocity field with an automatic data reduction system. This permits the reduction of large numbers of holograms (time steps) in a reasonable amount of time. The current version of the HCV, built for proof-of-concept tests, uses low-frame rate holographic cameras and a prototype of a new type of water tunnel. This water tunnel is a unique low-disturbance facility which has minimal wall effects on the flow. This paper presents the first flow field examined by the HCV, the two-dimensional von Karman vortex street downstream of an unswept circular cylinder. Key factors in the HCV are flow speed, spatial and temporal resolution required, measurement volume, film transport speed, and laser pulse length. The interactions between these factors are discussed.

  11. Holocinematographic velocimeter for measuring time-dependent, three-dimensional flows

    NASA Astrophysics Data System (ADS)

    Beeler, George B.; Weinstein, Leonard M.

    1987-06-01

    Two simulatneous, orthogonal-axis holographic movies are made of tracer particles in a low-speed water tunnel to determine the time-dependent, three-dimensional velocity field. This instrument is called a Holocinematographic Velocimeter (HCV). The holographic movies are reduced to the velocity field with an automatic data reduction system. This permits the reduction of large numbers of holograms (time steps) in a reasonable amount of time. The current version of the HCV, built for proof-of-concept tests, uses low-frame rate holographic cameras and a prototype of a new type of water tunnel. This water tunnel is a unique low-disturbance facility which has minimal wall effects on the flow. This paper presents the first flow field examined by the HCV, the two-dimensional von Karman vortex street downstream of an unswept circular cylinder. Key factors in the HCV are flow speed, spatial and temporal resolution required, measurement volume, film transport speed, and laser pulse length. The interactions between these factors are discussed.

  12. Origin of the spike-timing-dependent plasticity rule

    NASA Astrophysics Data System (ADS)

    Cho, Myoung Won; Choi, M. Y.

    2016-08-01

    A biological synapse changes its efficacy depending on the difference between pre- and post-synaptic spike timings. Formulating spike-timing-dependent interactions in terms of the path integral, we establish a neural-network model, which makes it possible to predict relevant quantities rigorously by means of standard methods in statistical mechanics and field theory. In particular, the biological synaptic plasticity rule is shown to emerge as the optimal form for minimizing the free energy. It is further revealed that maximization of the entropy of neural activities gives rise to the competitive behavior of biological learning. This demonstrates that statistical mechanics helps to understand rigorously key characteristic behaviors of a neural network, thus providing the possibility of physics serving as a useful and relevant framework for probing life.

  13. Random walks for spike-timing-dependent plasticity

    NASA Astrophysics Data System (ADS)

    Williams, Alan; Leen, Todd K.; Roberts, Patrick D.

    2004-08-01

    Random walk methods are used to calculate the moments of negative image equilibrium distributions in synaptic weight dynamics governed by spike-timing-dependent plasticity. The neural architecture of the model is based on the electrosensory lateral line lobe of mormyrid electric fish, which forms a negative image of the reafferent signal from the fish’s own electric discharge to optimize detection of sensory electric fields. Of particular behavioral importance to the fish is the variance of the equilibrium postsynaptic potential in the presence of noise, which is determined by the variance of the equilibrium weight distribution. Recurrence relations are derived for the moments of the equilibrium weight distribution, for arbitrary postsynaptic potential functions and arbitrary learning rules. For the case of homogeneous network parameters, explicit closed form solutions are developed for the covariances of the synaptic weight and postsynaptic potential distributions.

  14. Optimization of Time-Dependent Particle Tracing Using Tetrahedral Decomposition

    NASA Technical Reports Server (NTRS)

    Kenwright, David; Lane, David

    1995-01-01

    An efficient algorithm is presented for computing particle paths, streak lines and time lines in time-dependent flows with moving curvilinear grids. The integration, velocity interpolation and step-size control are all performed in physical space which avoids the need to transform the velocity field into computational space. This leads to higher accuracy because there are no Jacobian matrix approximations or expensive matrix inversions. Integration accuracy is maintained using an adaptive step-size control scheme which is regulated by the path line curvature. The problem of cell-searching, point location and interpolation in physical space is simplified by decomposing hexahedral cells into tetrahedral cells. This enables the point location to be done analytically and substantially faster than with a Newton-Raphson iterative method. Results presented show this algorithm is up to six times faster than particle tracers which operate on hexahedral cells yet produces almost identical particle trajectories.

  15. Ionization and dissociation dynamics of molecules in strong laser fields

    NASA Astrophysics Data System (ADS)

    Lai, Wei

    The fast advancement of ultrashort-pulsed high-intensity laser technology allows for generating an electric field equivalent to the Coulomb field inside an atom or a molecule (e.g., EC=5.14x109 V/cm at the 1s orbit radius a0=0.0529 nm of the hydrogen atom, which corresponds to an intensity of 3.54x1016 W/cm2). Atoms and molecules exposed in such a field will easily be ionized, as the external field is strong enough to remove the electrons from the core. This is usually referred to "strong field". Strong fields provide a new tool for studying the interaction of atoms and molecules with light in the nonlinear nonperturbative regime. During the past three decades, significant progress has been made in the strong field science. Today, most phenomena involving atoms in strong fields have been relatively well understood by the single-active-electron (SAE) approximation. However, the interpretation of these responses in molecules has encountered great difficulties. Not like atoms that only undergo excitation and ionization, various dissociation channels accompanying excitation and ionization can occur in molecules during the laser pulse interaction, which imparts further complexity to the study of molecules in strong fields. Previous studies have shown that molecules can behave significantly different from rare gas atoms in phenomena as simple as single and double ionization. Molecular dissociation following ionization also presents challenges in strong fields compared to what we have learned in the weak-field regime. This dissertation focuses on experimental studies on ionization and dissociation of some commonly-seen small molecules in strong laser fields. Previous work of molecules in strong fields will be briefly reviewed, particularly on some open questions about multiple dissociation channels, nonsequential double ionization, enhanced ionization and molecular alignment. The identification of various molecular dissociation channels by recent experimental technical

  16. Thermal relaxation of adsorbed atoms in an intense laser field

    NASA Astrophysics Data System (ADS)

    Arnoldus, Henk F.; van Smaalen, Sander; George, Thomas F.

    1986-11-01

    Adsorbed atoms on the surface of a harmonic lattice are immersed in a strong laser field. The optical Bloch equations are derived, which include the thermal relaxation and the coherent excitation of the adbond. This is accomplished by a transformation to dressed states, which diagonalizes the interaction with the laser. The single-phonon couplings are then understood as transitions between dressed states. The radiative contributions for arbitrarily strong fields are obtained in the master equation, and it is shown that the coherences with respect to the dressed states decay exponentially, due to the phonon relaxation. General properties of the competing phonon-induced redistribution and optical excitation of the level populations are presented, and exemplified by an explicit elaboration of a three-level system. The results are amenable to analytical evaluation once the interaction potential is prescribed, and extensions of the approach to include multiphonon processes are straightforward.

  17. Laser Plasma Particle Accelerators: Large Fields for Smaller Facility Sources

    SciTech Connect

    Geddes, Cameron G.R.; Cormier-Michel, Estelle; Esarey, Eric H.; Schroeder, Carl B.; Vay, Jean-Luc; Leemans, Wim P.; Bruhwiler, David L.; Cary, John R.; Cowan, Ben; Durant, Marc; Hamill, Paul; Messmer, Peter; Mullowney, Paul; Nieter, Chet; Paul, Kevin; Shasharina, Svetlana; Veitzer, Seth; Weber, Gunther; Rubel, Oliver; Ushizima, Daniela; Bethel, Wes; Wu, John

    2009-03-20

    Compared to conventional particle accelerators, plasmas can sustain accelerating fields that are thousands of times higher. To exploit this ability, massively parallel SciDAC particle simulations provide physical insight into the development of next-generation accelerators that use laser-driven plasma waves. These plasma-based accelerators offer a path to more compact, ultra-fast particle and radiation sources for probing the subatomic world, for studying new materials and new technologies, and for medical applications.

  18. Analytical model for calibrating laser intensity in strong-field-ionization experiments

    NASA Astrophysics Data System (ADS)

    Zhao, Song-Feng; Le, Anh-Thu; Jin, Cheng; Wang, Xu; Lin, C. D.

    2016-02-01

    The interaction of an intense laser pulse with atoms and molecules depends extremely nonlinearly on the laser intensity. Yet experimentally there still exists no simple reliable methods for determining the peak laser intensity within the focused volume. Here we present a simple method, based on an improved Perelomov-Popov-Terent'ev model, that would allow the calibration of laser intensities from the measured ionization signals of atoms or molecules. The model is first examined by comparing ionization probabilities (or signals) of atoms and several simple diatomic molecules with those from solving the time-dependent Schrödinger equation. We then show the possibility of using this method to calibrate laser intensities for atoms, diatomic molecules as well as large polyatomic molecules, for laser intensities from the multiphoton ionization to tunneling ionization regimes.

  19. Weibel magnetic field competes with Biermann fields in laser-solid interactions

    NASA Astrophysics Data System (ADS)

    Shukla, Nitin; Schoeffler, Kevin; Vieira, Jorge; Fonseca, Ricardo; Silva, Luis

    2016-10-01

    Biermann battery induced magnetic fields caused by non-parallel density and temperature gradients, first investigated experimentally, continue to be measured in many current experiments. A detailed study of Biermann generated magnetic fields in collisionless systems has been carried out, showing that for large system sizes (L /de >= 100) , where de is the electron inertial length, the Weibel instability dominates as the major source of magnetic field. In this work, we demonstrate the possibility of experimentally generating this strong Weibel magnetic field. We model, using ab initio PIC simulations, the interaction of a short (ps) high intensity (a0 >= 1) laser pulse, with a target of sufficiently large gradient scale length, L. The expanding hot energetic electron population generated by the laser produces an anisotropy in the velocity distribution. This anisotropy provides the free energy that drives the Weibel instability that appears on the surfaces of the target and dominates over the Biermann battery field.

  20. Angular radiation temperature simulation for time-dependent capsule drive prediction in inertial confinement fusion

    SciTech Connect

    Jing, Longfei; Yang, Dong; Li, Hang; Zhang, Lu; Lin, Zhiwei; Li, Liling; Kuang, Longyu; Jiang, Shaoen Ding, Yongkun; Huang, Yunbao

    2015-02-15

    The x-ray drive on a capsule in an inertial confinement fusion setup is crucial for ignition. Unfortunately, a direct measurement has not been possible so far. We propose an angular radiation temperature simulation to predict the time-dependent drive on the capsule. A simple model, based on the view-factor method for the simulation of the radiation temperature, is presented and compared with the experimental data obtained using the OMEGA laser facility and the simulation results acquired with VISRAD code. We found a good agreement between the time-dependent measurements and the simulation results obtained using this model. The validated model was then used to analyze the experimental results from the Shenguang-III prototype laser facility. More specifically, the variations of the peak radiation temperatures at different view angles with the albedo of the hohlraum, the motion of the laser spots, the closure of the laser entrance holes, and the deviation of the laser power were investigated. Furthermore, the time-dependent radiation temperature at different orientations and the drive history on the capsule were calculated. The results indicate that the radiation temperature from “U20W112” (named according to the diagnostic hole ID on the target chamber) can be used to approximately predict the drive temperature on the capsule. In addition, the influence of the capsule on the peak radiation temperature is also presented.

  1. Quantum-orbit analysis for yield and ellipticity of high order harmonic generation with elliptically polarized laser field.

    PubMed

    Li, Yang; Zhu, Xiaosong; Zhang, Qingbin; Qin, Meiyan; Lu, Peixiang

    2013-02-25

    We perform a quantum-orbit analysis for the dependence of high-order-harmonic yield on the driving field ellipticity and the polarization properties of the generated high harmonics. The electron trajectories responsible for the emission of particular harmonics are identified. It is found that, in elliptically polarized driving field, the electrons have ellipticity-dependent initial velocities, which lead to the decrease of the ionization rate. Thus the harmonic yield steeply decreases with laser ellipticity. Besides, we show that the polarization properties of the harmonics are related to the complex momenta of the electron. The physical origin of the harmonic ellipticity is interpreted as the consequence of quantum-mechanical uncertainty of the electron momentum. Our results are verified with the experimental results as well as the numerical solutions of the time dependent Schrödinger equation from the literature.

  2. Test field for airborne laser scanning in Finland

    NASA Astrophysics Data System (ADS)

    Ahokas, E.; Kaartinen, H.; Kukko, A.; Litkey, P.

    2014-11-01

    Airborne laser scanning (ALS) is a widely spread operational measurement tool for obtaining 3D coordinates of the ground surface. There is a need for calibrating the ALS system and a test field for ALS was established at the end of 2013. The test field is situated in the city of Lahti, about 100 km to the north of Helsinki. The size of the area is approximately 3.5 km × 3.2 km. Reference data was collected with a mobile laser scanning (MLS) system assembled on a car roof. Some streets were measured both ways and most of them in one driving direction only. The MLS system of the Finnish Geodetic Institute (FGI) consists of a navigation system (NovAtel SPAN GNSS-IMU) and a laser scanner (FARO Focus3D 120). In addition to the MLS measurements more than 800 reference points were measured using a Trimble R8 VRS-GNSS system. Reference points are along the streets, on parking lots, and white pedestrian crossing line corners which can be used as reference targets. The National Land Survey of Finland has already used this test field this spring for calibrating their Leica ALS-70 scanner. Especially it was easier to determine the encoder scale factor parameter using this test field. Accuracy analysis of the MLS points showed that the point height RMSE is 2.8 cm and standard deviation is 2.6 cm. Our purpose is to measure both more MLS data and more reference points in the test field area to get a better spatial coverage. Calibration flight heights are planned to be 1000 m and 2500 m above ground level. A cross pattern, southwest-northeast and northwest-southeast, will be flown both in opposite directions.

  3. Near-field and far-field engineering of semiconductor lasers

    NASA Astrophysics Data System (ADS)

    Yu, Nanfang

    Plasmonics focuses on the interaction between light and metallic films or nanostructures. In the last two decades, intensive research efforts were devoted to exploring the extremely broad applications of plasmonics. My research combines the versatility of plasmonics with active light sources, i.e., quantum cascade lasers (QCLs). This thesis focuses on the application of plasmonics in near-field and far-field engineering of semiconductor lasers, specifically, subwavelength focusing in the near-field, and laser beam collimation and polarization control. The first chapter of this thesis lays out fundamental materials necessary for understanding the following chapters. Systematic simulation and experimental results are presented in Chapter 2 to demonstrate that the integration of a suitably designed one dimensional or two dimensional plasmonic structures on the facet of QCLs can reduce the beam divergence by more than one order of magnitude. The devices with optimized collimators preserve a high output power, comparable to that of the unpatterned lasers. Chapter 3 demonstrates that the polarization state of the output of semiconductor lasers can be controlled by defining plasmonic structures on the laser facet. An integrated plasmonic polarizer can project the polarization of a semiconductor laser onto other directions. By patterning a facet with two orthogonal grating-aperture structures, a QCL can produce emission consisting of a superposition of a linearly and right-circularly polarized light, a first step towards a circularly-polarized laser. Chapter 4 presents experimental work on the coupled-rod antennas and the bowtie antennas patterned on the facet of QCLs. Both designs can provide an optical field confinement on the order of lambda/50 and with peak intensity on the order of 1 GW/cm2 in the antenna gap. The bowtie devices are more advanced due to better confinement of light into a single spot. Chapter 5 and 6 discuss two side research topics. Chapter 5

  4. Tomographic reconstruction of three-dimensional density fields using laser speckle photography and laser interferometry projections

    NASA Astrophysics Data System (ADS)

    Ko, Hanseo

    The reconstruction accuracies of Fourier convolution (FC) and algebraic reconstruction technique (ART) are examined for laser speckle photography and laser interferometry. Computer synthesized phantoms are used to calculate asymmetric density fields for limited cases of 5 and 3 projections. To simulate experimental uncertainties, random noise levels are imposed on projected data before they are used for reconstruction. Experiments are also performed for a speckle photography system, a Mach- Zehnder interferometer, and an oxygen analyzer for a half-blocked nozzle and a two-hole nozzle to measure asymmetric helium density fields. Reconstructed density fields are calculated by the FC and the ART from projected data of the speckle photography and the interferometry. The reconstructed fields are compared with the results of the directly measured data using oxygen analyzer. The non-algebraic ART requires a modification for its use for laser speckle photography. Both the ART and the FC have been used for both non- algebraic speckle photography and algebraic interferometry. The present ART method shows a significant improvement in the reconstruction accuracy over the existing Fourier convolution (FC) method.

  5. Exploration of strong-field double ionization of CS2 molecule in bichromatic counterrotating circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Ben, Shuai; Zuo, Wanlong; Song, Kaili; Xu, Tongtong; Guo, Jing; Xu, Haifeng; Yan, Bing; Liu, Xue-Shen

    2016-12-01

    By using classical ensemble method, we investigate the double ionization of CS2 molecule in linearly, the bichromatic counterrotating circularly polarized laser fields and the combination of bichromatic counterrotating circularly polarized laser fields and static field, respectively. The numerical results show that the ionization probability in the bichromatic counterrotating circularly polarized laser fields is about 2 order magnitude higher than that in linearly polarized laser field. When a static field is added, the ionization probability is the largest. Besides, the "knee" structure occurs at about 0.05 PW/cm2 in linearly polarized laser field; whereas "knee" structure is disappeared in the bichromatic counterrotating circularly polarized laser fields and combined laser field. The corresponding momentum distribution of CS2 molecule presents a "finger-like" structure at about 0.05 PW/cm2 in linearly polarized field. By analysing the energy distributions of double-ionized electrons versus time and corresponding trajectories, we find that, for linearly polarized case non-sequential double ionization (NSDI) is predominant at about 0.05 PW/cm2, for bichromatic counterrotating circularly polarized laser fields, one electron ionizes after another which indicate sequential ionization process (SDI). When the static field is added, the two electrons undergoes a long pre-ionization process first and then ionizes one after another, and the pre-ionization process lasts longer than other two cases.

  6. Field precision machining technology of target chamber in ICF lasers

    NASA Astrophysics Data System (ADS)

    Xu, Yuanli; Wu, Wenkai; Shi, Sucun; Duan, Lin; Chen, Gang; Wang, Baoxu; Song, Yugang; Liu, Huilin; Zhu, Mingzhi

    2016-10-01

    In ICF lasers, many independent laser beams are required to be positioned on target with a very high degree of accuracy during a shot. The target chamber provides a precision platform and datum reference for final optics assembly and target collimation and location system. The target chamber consists of shell with welded flanges, reinforced concrete pedestal, and lateral support structure. The field precision machining technology of target chamber in ICF lasers have been developed based on ShenGuangIII (SGIII). The same center of the target chamber is adopted in the process of design, fabrication, and alignment. The technologies of beam collimation and datum reference transformation are developed for the fabrication, positioning and adjustment of target chamber. A supporting and rotating mechanism and a special drilling machine are developed to bore the holes of ports. An adjustment mechanism is designed to accurately position the target chamber. In order to ensure the collimation requirements of the beam leading and focusing and the target positioning, custom-machined spacers are used to accurately correct the alignment error of the ports. Finally, this paper describes the chamber center, orientation, and centering alignment error measurements of SGIII. The measurements show the field precision machining of SGIII target chamber meet its design requirement. These information can be used on similar systems.

  7. Retrieval of target structure information from laser-induced photoelectrons by few-cycle bicircular laser fields

    NASA Astrophysics Data System (ADS)

    Hoang, Van-Hung; Le, Van-Hoang; Lin, C. D.; Le, Anh-Thu

    2017-03-01

    By analyzing theoretical results from a numerical solution of the time-dependent Schrödinger equation for atoms in few-cycle bicircular laser pulses, we show that high-energy photoelectron momentum spectra can be used to extract accurate elastic scattering differential cross sections of the target ion with free electrons. We find that the retrieval range for a scattering angle with bicircular pulses is wider than with linearly polarized pulses, although the retrieval method has to be modified to account for different returning directions of the electron in the continuum. This result can be used to extend the range of applicability of ultrafast imaging techniques such as laser-induced electron diffraction and for the accurate characterization of laser pulses.

  8. The Mitral Valve Prolapsus : Quantification of the Regurgitation Flow Rate by Experimental Time-Dependant PIV

    DTIC Science & Technology

    2007-11-02

    The Mitral Valve Prolapsus : Quantification of the Regurgitation Flow Rate by Experimental Time-Dependant PIV. F. Billy1, D. Coisne1,2, L. Sanchez1... mitral valve insufficiency), assumes that the velocity field in the convergent region have hemispheric shapes and introduce miscalculation specially...upstream a prolaps model of regurgitant orifice based on 2D time dependent PIV reconstruction. Keywords- Mitral Valve , Prolapsus, Regurgitation Flow

  9. Multiconfigurational time-dependent Hartree method for bosons: Many-body dynamics of bosonic systems

    NASA Astrophysics Data System (ADS)

    Alon, Ofir E.; Streltsov, Alexej I.; Cederbaum, Lorenz S.

    2008-03-01

    The evolution of Bose-Einstein condensates is amply described by the time-dependent Gross-Pitaevskii mean-field theory which assumes all bosons to reside in a single time-dependent one-particle state throughout the propagation process. In this work, we go beyond mean field and develop an essentially exact many-body theory for the propagation of the time-dependent Schrödinger equation of N interacting identical bosons. In our theory, the time-dependent many-boson wave function is written as a sum of permanents assembled from orthogonal one-particle functions, or orbitals, where both the expansion coefficients and the permanents (orbitals) themselves are time-dependent and fully determined according to a standard time-dependent variational principle. By employing either the usual Lagrangian formulation or the Dirac-Frenkel variational principle we arrive at two sets of coupled equations of motion, one for the orbitals and one for the expansion coefficients. The first set comprises of first-order differential equations in time and nonlinear integrodifferential equations in position space, whereas the second set consists of first-order differential equations with time-dependent coefficients. We call our theory multiconfigurational time-dependent Hartree for bosons, or MCTDHB(M) , where M specifies the number of time-dependent orbitals used to construct the permanents. Numerical implementation of the theory is reported and illustrative numerical examples of many-body dynamics of trapped Bose-Einstein condensates are provided and discussed. The convergence of the method with a growing number M of orbitals is demonstrated in a specific example of four interacting bosons in a double well.

  10. Enhancing molecular orientation by combining electrostatic and four-color laser fields

    NASA Astrophysics Data System (ADS)

    Xu, Shuwu; Yao, Yunhua; Lu, Chenhui; Jia, Tianqing; Ding, Jingxin; Zhang, Shian; Sun, Zhenrong

    2014-09-01

    We propose a scheme to enhance molecular orientation by combing an intense electrostatic field and a four-color laser field. We show that molecular orientation by the combined field can be obtained under a laser-field-free condition, and the maximal orientation degree can be enhanced by comparing with the sum of that individually created by the electrostatic field and the four-color laser field. Our results show that the orientation enhancement results from the larger asymmetry of the four-color laser field because of the existence of the electrostatic field. Furthermore, we also discuss the dependence of the orientation enhancement on the carrier-envelope phase, laser intensity, and pulse duration of the four-color laser field and the molecular rotational temperature.

  11. On precession of entangled spins in a strong laser field

    SciTech Connect

    Eliashvili, M.; Gerdt, V.; Khvedelidze, A.

    2009-05-15

    A dynamics of the entanglement under an environmental influence is modelled by a bound state composed of two heavy particles interacting with a strong laser. Adopting the semiclassical attitude, a trajectory of the bound state's center-of-mass is found from the Newton equations solved beyond the dipole approximation and taking into account the magnetic field effect. At the same time the dynamics of constituent spins under the laser coupling is studied quantum mechanically solving the nonrelativistic von Neumann equation with the effective Hamiltonian determined by the bound state's classical trajectory. Based on the solution, the effects of an intense linearly polarized monochromatic plane wave on the precession of entangled spins are discussed for a specific kind of mixed initial states including a family of maximally entangled Werner states.

  12. Annular billiard dynamics in a circularly polarized strong laser field

    NASA Astrophysics Data System (ADS)

    Kamor, A.; Mauger, F.; Chandre, C.; Uzer, T.

    2012-01-01

    We analyze the dynamics of a valence electron of the buckminsterfullerene molecule (C60) subjected to a circularly polarized laser field by modeling it with the motion of a classical particle in an annular billiard. We show that the phase space of the billiard model gives rise to three distinct trajectories: “whispering gallery orbits,” which hit only the outer billiard wall; “daisy orbits,” which hit both billiard walls (while rotating solely clockwise or counterclockwise for all time); and orbits that only visit the downfield part of the billiard, as measured relative to the laser term. These trajectories, in general, maintain their distinct features, even as the intensity is increased from 1010 to 1014Wcm-2. We attribute this robust separation of phase space to the existence of twistless tori.

  13. Laser ablation with applied magnetic field for electric propulsion

    NASA Astrophysics Data System (ADS)

    Batishcheva, Alla; Batishchev, Oleg; Cambier, Jean-Luc

    2012-10-01

    Using ultrafast lasers with tera-watt-level power allows efficient ablation and ionization of solid-density materials [1], creating dense and hot (˜100eV) plasma. We propose ablating small droplets in the magnetic nozzle configurations similar to mini-helicon plasma source [2]. Such approach may improve the momentum coupling compared to ablation of solid surfaces and facilitate plasma detachment. Results of 2D modeling of solid wire ablation in the applied magnetic field are presented and discussed. [4pt] [1] O. Batishchev et al, Ultrafast Laser Ablation for Space Propulsion, AIAA technical paper 2008-5294, -16p, 44th JPC, Hartford, 2008.[0pt] [2] O. Batishchev and J.L. Cambier, Experimental Study of the Mini-Helicon Thruster, Air Force Research Laboratory Report, AFRL-RZ-ED-TR-2009-0020, 2009.

  14. Investigating tunneling process of atom exposed in circularly polarized strong-laser field

    NASA Astrophysics Data System (ADS)

    Yuan, MingHu; Xin, PeiPei; Chu, TianShu; Liu, HongPing

    2017-03-01

    We propose a method for studying the tunneling process by analyzing the instantaneous ionization rate of a circularly polarized laser. A numerical calculation shows that, for an atom exposed to a long laser pulse, if its initial electronic state wave function is non-spherical symmetric, the delayed phase shift of the ionization rate vs the laser cycle period in real time in the region close to the peak intensity of the laser pulse can be used to probe the tunneling time. In this region, an obvious time delay phase shift of more than 190 attoseconds is observed. Further study shows that the atom has a longer tunneling time in the ionization under a shorter wavelength laser pulse. In our method, a Wigner rotation technique is employed to numerically solve the time-dependent Schrödinger equation of a single-active electron in a three-dimensional spherical coordinate system.

  15. Nonsequential Double Ionization of Atoms in Strong Laser Field: Identifying the Mechanisms behind the Correlated-Electron Momentum Spectra

    NASA Astrophysics Data System (ADS)

    Ye, Difa; Fu, Libin; Liu, Jie

    Within the strong-field physics community, there has been increasing interest on nonsequential double ionization (NSDI) induced by electron-electron (e-e) correlation. A large variety of novel phenomena has been revealed in experiments during the past decades. However, the theoretical understanding and interpretation of this process is still far from being complete. The most accurate simulation, i.e. the exact solution of the time-dependent Schrödinger equation (TDSE) for two electrons in a laser field is computationally expensive. In order to overcome the difficulty, we proposed a feasible semiclassical model, in which we treat the tunneling ionization of the outmost electron quantum mechanically according to the ADK theory, sample the inner electron from microcanonical distribution and then evolve the two electrons with Newton's equations. With this model, we have successfully explained various NSDI phenomena, including the excessive DI yield, the energy spectra and angular distribution of photoelectrons. Very recently, it is adopted to reveal the physical mechanisms behind the fingerlike structure in the correlated electron momentum spectra, the unexpected correlation-anticorrelation transition close to the recollision threshold, and the anomalous NSDI of alkaline-earth-metal atoms in circularly polarized field. The obvious advantage of our model is that it gives time-resolved insights into the complex dynamics of NSDI, from the turn-on of the laser field to the final escape of the electrons, thus allowing us to disentangle and thoroughly analyze the underlying physical mechanisms.

  16. Quantum control of molecular fragmentation in strong laser fields

    NASA Astrophysics Data System (ADS)

    Zohrabi, Mohammad

    Present advances in laser technology allow the production of ultrashort (<˜5 fs, approaching single cycle at 800 nm), intense tabletop laser pulses. At these high intensities laser-matter interactions cannot be described with perturbation theory since multiphoton processes are involved. This is in contrast to photodissociation by the absorption of a single photon, which is well described by perturbation theory. For example, at high intensities (<˜5x1013 W/cm2) the fragmentation of molecular hydrogen ions has been observed via the absorption of three or more photons. In another example, an intriguing dissociation mechanism has been observed where molecular hydrogen ions seem to fragment by apparently absorbing no photons. This is actually a two photon process, photoabsorption followed by stimulated emission, resulting in low energy fragments. We are interested in exploring these kinds of multiphoton processes. Our research group has studied the dynamics and control of fragmentation induced by strong laser fields in a variety of molecular targets. The main goal is to provide a basic understanding of fragmentation mechanisms and possible control schemes of benchmark systems such as H2+. This knowledge is further extended to more complex systems like the benchmark H3+ polyatomic and other molecules. In this dissertation, we report research based on two types of experiments. In the first part, we describe laser-induced fragmentation of molecular ion-beam targets. In the latter part, we discuss the formation of highly-excited neutral fragments from hydrogen molecules using ultrashort laser pulses. In carrying out these experiments, we have also extended experimental techniques beyond their previous capabilities. We have performed a few experiments to advance our understanding of laser-induced fragmentation of molecular-ion beams. For instance, we explored vibrationally resolved spectra of O2+ dissociation using various wavelengths. We observed a vibrational suppression

  17. Time-Resolved Spectroscopy in Time-Dependent Density Functional Theory: An Exact Condition

    NASA Astrophysics Data System (ADS)

    Fuks, Johanna I.; Luo, Kai; Sandoval, Ernesto D.; Maitra, Neepa T.

    2015-05-01

    A fundamental property of a quantum system driven by an external field is that when the field is turned off the positions of its response frequencies are independent of the time at which the field is turned off. We show that this leads to an exact condition for the exchange-correlation potential of time-dependent density functional theory. The Kohn-Sham potential typically continues to evolve after the field is turned off, which leads to time dependence in the response frequencies of the Kohn-Sham response function. The exchange-correlation kernel must cancel out this time dependence. The condition is typically violated by approximations currently in use, as we demonstrate by several examples, which has severe consequences for their predictions of time-resolved spectroscopy.

  18. Dynamics of emitting electrons in strong laser fields

    SciTech Connect

    Sokolov, Igor V.; Naumova, Natalia M.; Nees, John A.; Yanovsky, Victor P.; Mourou, Gerard A.

    2009-09-15

    A new derivation of the motion of a radiating electron is given, leading to a formulation that differs from the Lorentz-Abraham-Dirac equation and its published modifications. It satisfies the proper conservation laws. Particularly, it conserves the generalized momentum, eliminating the symmetry-breaking runaway solution. The equation allows a consistent calculation of the electron current, the radiation effect on the electron momentum, and the radiation itself, for a single electron or plasma electrons in strong electromagnetic fields. The equation is then applied to a simulation of a strong laser pulse interaction with a plasma target. Some analytical solutions are also provided.

  19. Laser Interferometer Space Antenna (LISA) Far Field Phase Pattern

    NASA Technical Reports Server (NTRS)

    Waluschka, Eugene

    1999-01-01

    The Laser Interferometry Space Antenna (LISA) for the detection of Gravitational Waves is a very long baseline interferometer that will measure the changes in the distance of a five million kilometer arm to pico meter accuracies. Knowledge of the phase deviations from a spherical wave and what causes these deviations are needed considerations in (as a minimum) the design of the telescope and in determining pointing requirements. Here we present the far field phase deviations from a spherical wave for given Zernike aberrations and obscurations of the exit pupil.

  20. Laser Interferometer Space Antenna (LISA) Far Field Phase Patterns

    NASA Technical Reports Server (NTRS)

    Waluschka, Eugene

    1999-01-01

    The Laser Interferometer Space Antenna (LISA) for the detection of Gravitational Waves is a very long baseline interferometer, which will measure the changes in the distance of a five million kilometer arm to picometer accuracies. Knowledge of the phase deviations from a spherical wave and what causes these deviations are needed considerations in (as a minimum) the design of the telescope and in determining pointing requirements. Here we will present the far field phase deviations from a spherical wave for given Zernike aberrations of the exit pupil and discuss how these results affect the choice of a telescope design.

  1. Anomalous Radiative Trapping in Laser Fields of Extreme Intensity

    NASA Astrophysics Data System (ADS)

    Gonoskov, A.; Bashinov, A.; Gonoskov, I.; Harvey, C.; Ilderton, A.; Kim, A.; Marklund, M.; Mourou, G.; Sergeev, A.

    2014-07-01

    We demonstrate that charged particles in a sufficiently intense standing wave are compressed toward, and oscillate synchronously at, the antinodes of the electric field. We call this unusual behavior anomalous radiative trapping (ART). We show using dipole pulses, which offer a path to increased laser intensity, that ART opens up new possibilities for the generation of radiation and particle beams, both of which are high energy, directed, and collimated. ART also provides a mechanism for particle control in high-intensity quantum-electrodynamics experiments.

  2. Wide-field Fourier ptychographic microscopy using laser illumination source

    PubMed Central

    Chung, Jaebum; Lu, Hangwen; Ou, Xiaoze; Zhou, Haojiang; Yang, Changhuei

    2016-01-01

    Fourier ptychographic (FP) microscopy is a coherent imaging method that can synthesize an image with a higher bandwidth using multiple low-bandwidth images captured at different spatial frequency regions. The method’s demand for multiple images drives the need for a brighter illumination scheme and a high-frame-rate camera for a faster acquisition. We report the use of a guided laser beam as an illumination source for an FP microscope. It uses a mirror array and a 2-dimensional scanning Galvo mirror system to provide a sample with plane-wave illuminations at diverse incidence angles. The use of a laser presents speckles in the image capturing process due to reflections between glass surfaces in the system. They appear as slowly varying background fluctuations in the final reconstructed image. We are able to mitigate these artifacts by including a phase image obtained by differential phase contrast (DPC) deconvolution in the FP algorithm. We use a 1-Watt laser configured to provide a collimated beam with 150 mW of power and beam diameter of 1 cm to allow for the total capturing time of 0.96 seconds for 96 raw FPM input images in our system, with the camera sensor’s frame rate being the bottleneck for speed. We demonstrate a factor of 4 resolution improvement using a 0.1 NA objective lens over the full camera field-of-view of 2.7 mm by 1.5 mm. PMID:27896016

  3. Quantum dynamics with fermion coupled coherent states: Theory and application to electron dynamics in laser fields

    SciTech Connect

    Kirrander, Adam; Shalashilin, Dmitrii V.

    2011-09-15

    We present an alternate version of the coupled-coherent-state method, specifically adapted for solving the time-dependent Schroedinger equation for multielectron dynamics in atoms and molecules. This theory takes explicit account of the exchange symmetry of fermion particles, and it uses fermion molecular dynamics to propagate trajectories. As a demonstration, calculations in the He atom are performed using the full Hamiltonian and accurate experimental parameters. Single- and double-ionization yields by 160-fs and 780-nm laser pulses are calculated as a function of field intensity in the range 10{sup 14}-10{sup 16} W/cm{sup 2}, and good agreement with experiments by Walker et al. is obtained. Since this method is trajectory based, mechanistic analysis of the dynamics is straightforward. We also calculate semiclassical momentum distributions for double ionization following 25-fs and 795-nm pulses at 1.5x10{sup 15} W/cm{sup 2}, in order to compare them with the detailed experiments by Rudenko et al. For this more challenging task, full convergence is not achieved. However, major effects such as the fingerlike structures in the momentum distribution are reproduced.

  4. Photoelectron momentum distributions of molecules in bichromatic circularly polarized attosecond UV laser fields

    NASA Astrophysics Data System (ADS)

    Yuan, Kai-Jun; Chelkowski, Szczepan; Bandrauk, André D.

    2016-05-01

    We theoretically investigate molecular photoelectron momentum distributions (MPMDs) by bichromatic [frequencies (ω1,ω2)] circularly polarized attosecond UV laser pulses. Simulations performed on aligned single-electron H2+ by numerically solving the corresponding three-dimensional time-dependent Schrödinger equation within a static nucleus frame show that MPMDs exhibit a spiral structure for both co-rotating and counter-rotating schemes. Results are analyzed by attosecond perturbation ionization models. Coherent electron wave packets created, respectively, by the two color pulses in the continuum interfere with each other. Photoionization distributions are functions of the photoelectron momentum p and the ejection angle θ , thus leading to spiral MPMDs. The dependence of spiral MPMDs on the time delay between the bicircular pulses and their relative phases is also presented. The spiral interference patterns are determined by the helicities and frequencies (ω1,ω2 ) of the bicircular fields. It is also found that the spiral patterns are sensitive to the molecular alignment and suppressed by two-center ionization interference, thus offering new tools for imaging molecular geometry.

  5. Experimental quantum-walk revival with a time-dependent coin.

    PubMed

    Xue, P; Zhang, R; Qin, H; Zhan, X; Bian, Z H; Li, J; Sanders, Barry C

    2015-04-10

    We demonstrate a quantum walk with time-dependent coin bias. With this technique we realize an experimental single-photon one-dimensional quantum walk with a linearly ramped time-dependent coin flip operation and thereby demonstrate two periodic revivals of the walker distribution. In our beam-displacer interferometer, the walk corresponds to movement between discretely separated transverse modes of the field serving as lattice sites, and the time-dependent coin flip is effected by implementing a different angle between the optical axis of half-wave plate and the light propagation at each step. Each of the quantum-walk steps required to realize a revival comprises two sequential orthogonal coin-flip operators, with one coin having constant bias and the other coin having a time-dependent ramped coin bias, followed by a conditional translation of the walker.

  6. Analytic description of high-order harmonic generation by atoms in a two-color laser field

    SciTech Connect

    Frolov, M. V.; Manakov, N. L.; Silaev, A. A.; Vvedenskii, N. V.

    2010-06-15

    A closed-form analytic formula describing high-order harmonic generation (HHG) in a two-color field of frequencies {omega} and 2{omega} is derived quantum mechanically in the low-frequency (tunneling) limit for an electron bound by a short-range potential and generalized to the case of an active electron in a neutral atom. The HHG rates are presented as a product of an electron wave packet describing the ionization of an active electron and its propagation in a laser field up to the recombination event and an atom-specific cross section of the electron's photorecombination. In contrast to the case of a monochromatic laser pulse [Frolov et al., Phys. Rev. Lett. 102, 243901 (2009)], the two-color wave packet involves the interference of two terms (involving the Airy function) that describe the emission of harmonics during the first and second half-cycles of the fundamental laser cycle and give rise to the two-plateau structures in the HHG spectra. For the case of the H atom, we show that our analytic results are in good agreement with those obtained from a numerical solution of the three-dimensional time-dependent Schroedinger equation. The factorization formula is used for describing the dependence of HHG rates for inert gases on the relative phase and intensities of the {omega} and 2{omega} components of a laser field. It is shown that atomic structure (including electron correlation) effects can modify substantially the two-color HHG spectra of inert gases.

  7. Coherent control of D2/H2 dissociative ionization by a mid-infrared two-color laser field

    NASA Astrophysics Data System (ADS)

    Wanie, Vincent; Ibrahim, Heide; Beaulieu, Samuel; Thiré, Nicolas; Schmidt, Bruno E.; Deng, Yunpei; Alnaser, Ali S.; Litvinyuk, Igor V.; Tong, Xiao-Min; Légaré, François

    2016-01-01

    Steering the electrons during an ultrafast photo-induced process in a molecule influences the chemical behavior of the system, opening the door to the control of photochemical reactions and photobiological processes. Electrons can be efficiently localized using a strong laser field with a well-designed temporal shape of the electric component. Consequently, many experiments have been performed with laser sources in the near-infrared region (800 nm) in the interest of studying and enhancing the electron localization. However, due to its limited accessibility, the mid-infrared (MIR) range has barely been investigated, although it allows to efficiently control small molecules and even more complex systems. To push further the manipulation of basic chemical mechanisms, we used a MIR two-color (1800 and 900 nm) laser field to ionize H2 and D2 molecules and to steer the remaining electron during the photo-induced dissociation. The study of this prototype reaction led to the simultaneous control of four fragmentation channels. The results are well reproduced by a theoretical model solving the time-dependent Schrödinger equation for the molecular ion, identifying the involved dissociation mechanisms. By varying the relative phase between the two colors, asymmetries (i.e., electron localization selectivity) of up to 65% were obtained, corresponding to enhanced or equivalent levels of control compared to previous experiments. Experimentally easier to implement, the use of a two-color laser field leads to a better electron localization than carrier-envelope phase stabilized pulses and applying the technique in the MIR range reveals more dissociation channels than at 800 nm.

  8. Time-dependent potential-functional embedding theory

    SciTech Connect

    Huang, Chen; Libisch, Florian; Carter, Emily A.

    2014-03-28

    We introduce a time-dependent potential-functional embedding theory (TD-PFET), in which atoms are grouped into subsystems. In TD-PFET, subsystems can be propagated by different suitable time-dependent quantum mechanical methods and their interactions can be treated in a seamless, first-principles manner. TD-PFET is formulated based on the time-dependent quantum mechanics variational principle. The action of the total quantum system is written as a functional of the time-dependent embedding potential, i.e., a potential-functional formulation. By exploiting the Runge-Gross theorem, we prove the uniqueness of the time-dependent embedding potential under the constraint that all subsystems share a common embedding potential. We derive the integral equation that such an embedding potential needs to satisfy. As proof-of-principle, we demonstrate TD-PFET for a Na{sub 4} cluster, in which each Na atom is treated as one subsystem and propagated by time-dependent Kohn-Sham density functional theory (TDDFT) using the adiabatic local density approximation (ALDA). Our results agree well with a direct TDDFT calculation on the whole Na{sub 4} cluster using ALDA. We envision that TD-PFET will ultimately be useful for studying ultrafast quantum dynamics in condensed matter, where key regions are solved by highly accurate time-dependent quantum mechanics methods, and unimportant regions are solved by faster, less accurate methods.

  9. Time-dependent potential-functional embedding theory.

    PubMed

    Huang, Chen; Libisch, Florian; Peng, Qing; Carter, Emily A

    2014-03-28

    We introduce a time-dependent potential-functional embedding theory (TD-PFET), in which atoms are grouped into subsystems. In TD-PFET, subsystems can be propagated by different suitable time-dependent quantum mechanical methods and their interactions can be treated in a seamless, first-principles manner. TD-PFET is formulated based on the time-dependent quantum mechanics variational principle. The action of the total quantum system is written as a functional of the time-dependent embedding potential, i.e., a potential-functional formulation. By exploiting the Runge-Gross theorem, we prove the uniqueness of the time-dependent embedding potential under the constraint that all subsystems share a common embedding potential. We derive the integral equation that such an embedding potential needs to satisfy. As proof-of-principle, we demonstrate TD-PFET for a Na4 cluster, in which each Na atom is treated as one subsystem and propagated by time-dependent Kohn-Sham density functional theory (TDDFT) using the adiabatic local density approximation (ALDA). Our results agree well with a direct TDDFT calculation on the whole Na4 cluster using ALDA. We envision that TD-PFET will ultimately be useful for studying ultrafast quantum dynamics in condensed matter, where key regions are solved by highly accurate time-dependent quantum mechanics methods, and unimportant regions are solved by faster, less accurate methods.

  10. Conformation change of enzyme molecules in laser radiation field

    NASA Astrophysics Data System (ADS)

    Leshenyuk, N. S.; Prigun, M. V.; Apanasevitsh, E. E.; Kruglik, G. S.

    2007-06-01

    As a result of an analysis of macromolecules properties in the coherent optical radiation field and with allowance for the experimentally obtained unique data on the interaction of lazer radiation with biomolecules (dependence of the interaction efficiency on the coherence length, presence of the effect in the spectra region far from the absorption band), a mechanism of wave interaction is developed. Using this mathematical model, the calculations of a change in the macromolecules oscillatory energy in the coherent radiation field are performed. It is shown that the increase of macromolecules oscillatory energy depends strongly on the coherence length of radiation. On exposure to noncoherent radiation, the biomolecules oscillatory energy practically does not change, whereas on exposure to laser radiation (coherence length ~3 cm), energy of oscillations of atoms increases by an order of 2÷4, which results in a change in the conformation of biomolecules and activity of enzymes. Recently a lot of data are received concerning the change of lysosomal enzymes activity in blood plasma under action of laser radiation.

  11. Dynamics of strong-field laser-induced microplasma formation in noble gases

    SciTech Connect

    Romanov, D. A.; Compton, R.; Filin, A.; Levis, R. J.

    2010-03-15

    The ultrafast dynamics of microplasmas generated by femtosecond laser pulses in noble gases has been investigated using four-wave mixing (FWM). The time dependence of the FWM signal is observed to reach higher intensity levels faster for Xe, with progressively lower scattering intensity and longer time dynamics for the noble gas series Xe, Kr, Ar, Ne, and He. The temporal dynamics is interpreted in terms of a tunnel ionization and impact cooling mechanism. A formalism to interpret the observed phenomena is presented here with comparison to the measured laser intensity and gas pressure trends.

  12. Computational model for time development of the EM field in pulsed laser systems

    NASA Astrophysics Data System (ADS)

    Skrabelj, D.; Marincek, M.; Drevensek-Olenik, I.; Leskovar, M.; Copic, M.

    2007-05-01

    A computational model, which describes EM field formation in a pulsed laser from a randomly generated initial spontaneous field inside the laser cavity has been developed. The model is based on a two-dimensional fast Fourier transform and describes a real laser system taking into account a lensing and a diaphragm effect of the laser rod. The laser cavity is described by five effective planes, which represent different laser cavity elements-the back and the front mirror, the Q-switch element and the laser rod. At each plane the EM field is calculated in real space and propagation between the planes is achieved in Fourier space by multiplication with an appropriate phase factor. The computational time needed for simulation of a realistic pulse formation is in order of minutes. The model can predict the shape and the integral energy of the pulse, its transverse profile at different distances from the front mirror (including near and far field) and beam divergence. The results of the model were found to be in good agreement with measured parameters for a Q-switched ruby laser system running in stable as well as unstable cavity configurations. The temporal shape of a laser pulse was measured and calculated not only for the ruby laser, but also for a Nd:YAG laser. It was found that FWHM of a pulse produced by ruby laser is three times longer than FWHM of a pulse produced by Nd:YAG laser.

  13. Knee structure in double ionization of noble atoms in circularly polarized laser fields

    NASA Astrophysics Data System (ADS)

    Chen, Xiang; Wu, Yan; Zhang, Jingtao

    2017-01-01

    Nonsequential double ionization is characterized by a knee structure in the plot of double-ionization probability versus laser intensity. In circularly polarized (CP) laser fields, this structure has only been observed for Mg atoms. By choosing laser fields according to a scaling law, we exhibit the knee structure in CP laser fields for Ar and He atoms. The collision of the ionized electron with the core enhances the ionization of the second electron and forms the knee structure. The electron recollision is universal in CP laser fields, but the ionization probability in the knee region decreases as the wavelength of the driven field increases. For experimental observations, it is beneficial to use target atoms with small ionization potentials and laser fields with short wavelengths.

  14. X-ray scattering by atoms and molecules dressed with strong fs laser fields

    NASA Astrophysics Data System (ADS)

    Hertlein, Marcus; Belkacem, Ali; Prior, Michael; Feinberg, Benedict; Roesch, Juergen; Maddi, Jason; Glover, T. Ernest; Ackerman, Glenn

    2002-05-01

    We set up an experiment at the Advanced Light Source to study fs laser-induced modifications to the resulting charge state distribution of argon ions after a K-shell is removed by a synchrotron radiation x-ray. Measurements of the "laser-off" charge state distribution of Ar ions following Auger relaxation show very clear post collision interaction effects in agreement with results found in the literature. Our "laser-on" measurements of the charge state distribution of ions, with the laser is overlapped in time (100 ps) and space (< 0.1 mm) with the ALS x-ray pulse, show an unexpected time dependence, on the nano second time scale, of the electron yield correlated to high charge states. These results will be discussed.

  15. Variational analysis of Er : Ti : LiNbO 3 waveguide lasers based on Gaussian/two-half Gaussian mode field distribution

    NASA Astrophysics Data System (ADS)

    Zhang, De-Long; Wu, Bo

    2002-02-01

    Starting with two dimensional, scalar wave equation, a variational equation was established for the fundamental TE and TM modes guided in Ti : LiNbO 3 waveguides on the basis of assuming a symmetric Gaussian mode field function in the width direction and two-half Gaussian trial functions in the depth direction. The controllable waveguide fabrication parameters, including channel width, diffusion temperature, initial Ti-strip thickness and diffusion time, dependent of fundamental mode size, effective pump area, coupling efficiency between pump and laser modes, and the coupling loss between a Ti : LiNbO 3 waveguide and a fiber were numerically calculated for Z-cut Er : Ti : LiNbO 3 channel waveguide lasers at three possible emission wavelengths 1532,1563 and 1576 nm and two possible pump wavelengths 1480 and 980 nm. The calculated results were compared with those of Gaussian/Hermite-Gaussian mode field distribution in detail.

  16. A History of Spike-Timing-Dependent Plasticity

    PubMed Central

    Markram, Henry; Gerstner, Wulfram; Sjöström, Per Jesper

    2011-01-01

    How learning and memory is achieved in the brain is a central question in neuroscience. Key to today’s research into information storage in the brain is the concept of synaptic plasticity, a notion that has been heavily influenced by Hebb's (1949) postulate. Hebb conjectured that repeatedly and persistently co-active cells should increase connective strength among populations of interconnected neurons as a means of storing a memory trace, also known as an engram. Hebb certainly was not the first to make such a conjecture, as we show in this history. Nevertheless, literally thousands of studies into the classical frequency-dependent paradigm of cellular learning rules were directly inspired by the Hebbian postulate. But in more recent years, a novel concept in cellular learning has emerged, where temporal order instead of frequency is emphasized. This new learning paradigm – known as spike-timing-dependent plasticity (STDP) – has rapidly gained tremendous interest, perhaps because of its combination of elegant simplicity, biological plausibility, and computational power. But what are the roots of today’s STDP concept? Here, we discuss several centuries of diverse thinking, beginning with philosophers such as Aristotle, Locke, and Ribot, traversing, e.g., Lugaro’s plasticità and Rosenblatt’s perceptron, and culminating with the discovery of STDP. We highlight interactions between theoretical and experimental fields, showing how discoveries sometimes occurred in parallel, seemingly without much knowledge of the other field, and sometimes via concrete back-and-forth communication. We point out where the future directions may lie, which includes interneuron STDP, the functional impact of STDP, its mechanisms and its neuromodulatory regulation, and the linking of STDP to the developmental formation and continuous plasticity of neuronal networks. PMID:22007168

  17. Solving Time-Dependent Equations of SCHRÖDINGER-TYPE Using Mapped Infinite Elements

    NASA Astrophysics Data System (ADS)

    Duque, Jairo

    We present a general technique to solve one-dimensional time-dependent Schrödinger-type equations. A mapped infinite elements approach is used to eliminate spurious reflections of outgoing wave packets from the boundaries of the interval of interest. This procedure leads to more precise solutions because the space coordinates are discretized to approximate the solution in the entire physical domain. We show its utility giving numerical results on three typical examples: a bounded short-range potential; the unbounded potential of a particle in a dc field; and a Hamiltonian with an intrinsic time dependence like the Hamiltonian of a charged particle in an ac electromagnetic field.

  18. Resonant enhancement for amplitude-modulated laser filament induced magnetic field in an inhomogeneous plasma

    NASA Astrophysics Data System (ADS)

    Annou, R.; Tripathi, V. K.; Srivastava, M. P.

    1996-09-01

    The Tripathi-Liu [Phys. Plasmas 1, 990 (1994)] model of magnetic-field generation due to an amplitude-modulated laser in a plasma is revisited. At plasma resonance, where modulation frequency equals the plasma frequency, significant enhancement in the magnetic field is seen. The magnetic field is found to scale directly with laser intensity and plasma frequency, while scaling inversely with laser spot size.

  19. Time Dependent Studies of Reactive Shocks in the Gas Phase

    DTIC Science & Technology

    1978-11-16

    1 LEVEL NRL Memorandum Report 3W tO Time Dependent Studies of Reactive Shocks in the Gas Phase E.S. ORAN, ’T.R. YOUNG and J.P. BORIS Laboratory for...34-• TIME DEPENDENT STUDIES OF REACTIVE SHOCKS IN THE GAS PHASE I. Introduction This paper presents results obtained from a detailed numerical...chemical kinetics, reaction products, and intermediates produced in reactive gas mixtures ignited by the propagation of a shock front. The model is based

  20. One Dimensional Time-Dependent Tunnelling of Excitons

    NASA Astrophysics Data System (ADS)

    Kilcullen, Patrick; Salayka-Ladouceur, Logan; Malmgren, Kevin; Reid, Matthew; Shegelski, Mark R. A.

    2017-03-01

    We study the time-dependent tunnelling of excitons in one dimension using numerical integration based on the Crank-Nicholson method. A complete development of the time-dependent simulator is provided. External barriers studied include single and double delta barriers. We find that the appearance of transmission resonances depends strongly on the dielectric constant, relative effective masses, and initial spatial spread of the wavefunction. A discussion regarding applications to realistic systems is provided.

  1. Multiconfigurational Time-Dependent Hartree Methods for Bosonic Systems:. Theory and Applications

    NASA Astrophysics Data System (ADS)

    Alon, Ofir E.; Streltsov, Alexej I.; Sakmann, Kaspar; Cederbaum, Lorenz S.

    2013-02-01

    We review the multiconfigurational time-dependent Hartree method for bosons, which is a formally exact many-body theory for the propagation of the time dependent Schrödinger equation of N interacting identical bosons. In this approach, the time-dependent many-boson wavefunction is written as a sum of all permanents assembled from M orthogonal orbitals, where both the expansion coefficients and the permanents (orbitals) themselves are time-dependent and determined according to the Dirac-Frenkel time-dependent variational principle. In this way, a much larger effective subspace of the many-boson Hilbert space can be spanned in practice, in contrast to multiconfigurational expansions with timeindependent configurations. We also briefly discuss the extension of this method to bosonic mixtures and resonantly coupled bosonic atoms and molecules. Two applications in one dimension are presented: (i) the numerically exact solution of the time-dependent many-boson Schrödinger equation for the population dynamics in a repulsive bosonic Josephson junction is shown to deviate significantly from the predictions of the commonly used Gross-Pitaevskii equation and Bose-Hubbard model; and (ii) the many-body dynamics of a soliton train in an attractive Bose-Einstein condensate is shown to deviate substantially from the widely accepted predictions of the Gross--Pitaevskii mean-field theory.

  2. Elimination of collisional dephasing by control laser fields

    NASA Astrophysics Data System (ADS)

    Sokolov, Alexei

    2003-05-01

    The perturbation of electronic states during a molecular collision results in an adiabatic shift of natural molecular frequencies. It is this frequency shift (integrated over the collision time) that produces an oscillation phase shift, and ultimately leads to dephasing of a molecular ensemble. However, the fact that during the collision all molecular levels shift in unison can be used to eliminate the shift of one selected transition, by applying a control laser field to an adjacent (control) transition. The amplitude and frequency of the control field can be adjusted such that the time-varying Stark shift produced by this field precisely compensates collisional frequency shift for the transition of interest, and as a result suppresses dephasing. This technique can possibly be extended to adiabatic atomic collisions, and to different types of inhomogeneous broadening. Earlier workers have demonstrated similar methods for Doppler width reduction, by utilizing velocity-dependent Stark shifts produced by control fields. There is also a relation of this proposal to electromagnetically induced transparency.

  3. Modeling lidar waveforms with time-dependent stochastic radiative transfer theory for remote estimations of forest structure

    NASA Astrophysics Data System (ADS)

    Kotchenova, Svetlana Y.; Shabanov, Nikolay V.; Knyazikhin, Yuri; Davis, Anthony B.; Dubayah, Ralph; Myneni, Ranga B.

    2003-08-01

    Large footprint waveform-recording laser altimeters (lidars) have demonstrated a potential for accurate remote sensing of forest biomass and structure, important for regional and global climate studies. Currently, radiative transfer analyses of lidar data are based on the simplifying assumption that only single scattering contributes to the return signal, which may lead to errors in the modeling of the lower portions of recorded waveforms in the near-infrared spectrum. In this study we apply time-dependent stochastic radiative transfer (RT) theory to model the propagation of lidar pulses through forest canopies. A time-dependent stochastic RT equation is formulated and solved numerically. Such an approach describes multiple scattering events, allows for realistic representation of forest structure including foliage clumping and gaps, simulates off-nadir and multiangular observations, and has the potential to provide better approximations of return waveforms. The model was tested with field data from two conifer forest stands (southern old jack pine and southern old black spruce) in central Canada and two closed canopy deciduous forest stands (with overstory dominated by tulip poplar) in eastern Maryland. Model-simulated signals were compared with waveforms recorded by the Scanning Lidar Imager of Canopies by Echo Recovery (SLICER) over these regions. Model simulations show good agreement with SLICER signals having a slow decay of the waveform. The analysis of the effects of multiple scattering shows that multiply scattered photons magnify the amplitude of the reflected signal, especially that originating from the lower portions of the canopy.

  4. A modular method to handle multiple time-dependent quantities in Monte Carlo simulations

    NASA Astrophysics Data System (ADS)

    Shin, J.; Perl, J.; Schümann, J.; Paganetti, H.; Faddegon, B. A.

    2012-06-01

    A general method for handling time-dependent quantities in Monte Carlo simulations was developed to make such simulations more accessible to the medical community for a wide range of applications in radiotherapy, including fluence and dose calculation. To describe time-dependent changes in the most general way, we developed a grammar of functions that we call ‘Time Features’. When a simulation quantity, such as the position of a geometrical object, an angle, a magnetic field, a current, etc, takes its value from a Time Feature, that quantity varies over time. The operation of time-dependent simulation was separated into distinct parts: the Sequence samples time values either sequentially at equal increments or randomly from a uniform distribution (allowing quantities to vary continuously in time), and then each time-dependent quantity is calculated according to its Time Feature. Due to this modular structure, time-dependent simulations, even in the presence of multiple time-dependent quantities, can be efficiently performed in a single simulation with any given time resolution. This approach has been implemented in TOPAS (TOol for PArticle Simulation), designed to make Monte Carlo simulations with Geant4 more accessible to both clinical and research physicists. To demonstrate the method, three clinical situations were simulated: a variable water column used to verify constancy of the Bragg peak of the Crocker Lab eye treatment facility of the University of California, the double-scattering treatment mode of the passive beam scattering system at Massachusetts General Hospital (MGH), where a spinning range modulator wheel accompanied by beam current modulation produces a spread-out Bragg peak, and the scanning mode at MGH, where time-dependent pulse shape, energy distribution and magnetic fields control Bragg peak positions. Results confirm the clinical applicability of the method.

  5. Control of plasmon fields via irreversible ultrafast dynamics caused by interaction of infrared laser pulses with quantum-dot-metallic-nanoparticle molecules

    NASA Astrophysics Data System (ADS)

    Sadeghi, S. M.; Wing, W. J.; Gutha, R. R.

    2015-08-01

    We study irreversible ultrafast dynamics caused by interaction of a semiconductor quantum-dot-metallic-nanorod system with an infrared laser field. We show that when this system supports exciton-plasmon coupling, by just varying the amplitude of this laser for a short period of time (several nanoseconds), one can decide the instance when the plasmon field of the nanorod becomes significant and its duration. This is done by showing that a sudden rise in the amplitude of the infrared laser (positive pulse) can induce irreversible transition from one of the collective molecular states of this system to another, making the plasmon field significant. When this amplitude reduces for a short period of time (negative pulse), the system returns back to its initial state, suppressing this field. We provide a detailed description of how, depending on the location, the infrared-induced dynamics can lend itself to different time-dependent plasmon fields around the nanorod. Our results show that at a given moment of time at each location we can have dramatically different types of dynamics for the phase and amplitude of the plasmon field. Using these we show that a quantum-dot-metallic-nanoparticle system can act as an all-optical and logic gate.

  6. Real-time full field laser Doppler imaging

    NASA Astrophysics Data System (ADS)

    Leutenegger, Marcel; Harbi, Pascal; Thacher, Tyler; Raffoul, Wassim; Lasser, Theo

    2012-06-01

    We present a full field laser Doppler imaging instrument that enables real-time in vivo assessment of blood flow in dermal tissue and skin. The instrument monitors the blood perfusion in an area of about 50cm2 with 480 × 480 pixels per frame at a rate of 12-14 frames per second. Smaller frames can be monitored at much higher frame rates. We recorded the microcirculation in healthy skin before, during and after arterial occlusion. In initial clinical case studies, we imaged the microcirculation in burned skin and monitored the recovery of blood flow in a skin flap during reconstructive surgery indicating the high potential of LDI for clinical applications.

  7. Self-fields in free-electron lasers

    SciTech Connect

    Roberson, C.W.; Hafizi, B.

    1995-12-31

    We have analyzed the free-electron laser (FEL) interaction in the high gain Compton regime. The theory has been extended to include self field effects on FEL operation. These effects are particularly important in compact, low voltage FELs. The theory applies to the case where the optical beam is guided by the electron beam by gain focusing and maintains a constant profile through the wiggler. The finite-emittance electron beam, in turn, is matched to the wiggler. The bitatron motion of the electrons is determined by (i) the focusing force due to wiggler gradients and, (ii) the repulsive force due to self-fields. Based on the single-electron equations, it can be shown that self-field forces tend to increase the period of transverse oscillations of electrons in the wiggler. In the limit, the flow of electrons is purely laminar, with a uniform axial velocity along and across the wiggler resulting in an improved beam quality. We shall also discuss the effects of beam compression on growth rate.

  8. Time-dependent Brittle Deformation in Etna Basalt

    NASA Astrophysics Data System (ADS)

    Heap, M. J.; Baud, P.; Meredith, P. G.; Vinciguerra, S.; Bell, A. F.; Main, I. G.

    2008-12-01

    Mt Etna is the largest and most active volcano in Europe. Due to the high permeability of its volcanic rocks, the volcanic edifice hosts one of the biggest hydrogeologic reservoirs of Sicily (Ogniben, 1966). Pre-eruptive patterns of flank eruptions, closely monitored by means of ground deformation and seismicity, revealed the slow development of fracture systems at different altitudes, marked by repeated bursts of seismicity and accelerating/decelerating deformation patterns acting over the scale of months to days. The presence of a fluid phase in cracks within rock has been shown to dramatically affect both mechanical and chemical interactions. Chemically, it promotes time-dependent brittle deformation through such mechanisms as stress corrosion cracking that allows rocks to deform at stresses far below their short-term failure strength. Such crack growth is highly non-linear and accelerates towards dynamic failure over extended periods of time, even under constant applied stress; a phenomenon known as 'brittle creep'. Stress corrosion is considered to be responsible for the acceleratory cracking and seismicity prior to volcanic eruptions and is invoked as an important mechanism in forecasting models. Here we report results from a study of time-dependent brittle creep in water-saturated samples of Etna basalt (EB) under triaxial stress conditions (confining pressure of 50 MPa and pore fluid pressure of 20 MPa). Samples of EB were loaded at a constant strain rate of 10-5 s-1 to a pre-determined percentage of the short- term strength and left to deform under constant stress until failure. Crack damage evolution was monitored throughout each experiment by measuring the independent damage proxies of axial strain, pore volume change and output of acoustic emission (AE) energy, during brittle creep of creep strain rates ranging over four orders of magnitude. Our data demonstrate that the applied differential stress exerts a crucial influence on both time-to-failure and

  9. Laser Interferometer Space Antenna (LISA) Far Field Phase Patterns

    NASA Technical Reports Server (NTRS)

    Waluschka, Eugene; Obenschain, Arthur F. (Technical Monitor)

    2000-01-01

    The Laser Interferometer Space Antenna (LISA) consists of three spacecraft in orbit about the sun. The orbits are chosen such that the three spacecraft are always at (roughly) the vertices of a equilateral triangle with 5 million kilometer leg lengths. Even though the distances between the three spacecraft are 5 million kilometers, the expected phase shifts between any two beams, due to a gravitational wave, only correspond to a distance change of about 10 pico meters, which is about 10(exp -5) waves for a laser wavelength of 1064 nm. To obtain the best signal-to-noise ratio, noise sources such as changes in the apparent distances due to pointing jitter must be controlled carefully. This is the main reason for determining the far-field phase patterns of a LISA type telescope. Because of torque on the LISA spacecraft and other disturbances, continuous adjustments to the pointing of the telescopes are required. These pointing adjustments will be a "jitter" source. If the transmitted wave is perfectly spherical then rotations (Jitter) about its geometric center will not produce any effect at the receiving spacecraft. However, if the outgoing wave is not perfectly spherical, then pointing jitter will produce a phase variation at the receiving spacecraft. The following sections describe the "brute force" computational approach used to determine the scalar wave front as a function of exit pupil (Zernike) aberrations and to show the results (mostly graphically) of the computations. This approach is straightforward and produces believable phase variations to sub-pico meter accuracy over distances on the order of 5 million kilometers. As such this analyzes the far field phase sensitivity to exit pupil aberrations.

  10. Birefringence of Polymer Solutions in Time-Dependent Flows.

    NASA Astrophysics Data System (ADS)

    Geffroy-Aguilar, Enrique

    1990-01-01

    This is a study of changes of conformation of macromolecules in polymeric solutions which are subjected to time-dependent extensional flows generated by a two -roll mill flow device. The flows produced by the two-roll mill are linear, and two-dimensional. It has a stagnation point at the center of the flow field where the magnitudes of the strain-rates are greater than the vorticity. This study of conformational changes is based on data around the vicinity of the stagnation point, I for steady state flows, and several transient flow histories such as start -up, cessation, and double-step flows. We also present an analytical solution for the creeping flow generated by an infinitely long two-roll mill embedded in an unbounded fluid. This solution is used as a benchmark to compare the behavior of the polymer solutions when subjected to flows with different values for the ratio of rate-of-strain to vorticity. The conformational changes are determined experimentally using the Two-color Flow-Birefringence which provides an instantaneous and point-wise measure of the anisotropy of the fluid, together with the relative orientation of the anisotropy with respect to the principal axes of the flow field. Based on relaxation of the fluid anisotropy the characteristic time-scales of the polymer have been evaluated as a function of the flow field properties and the degree of conformational change of the macromolecules. Data for two polymeric solutions is presented. The first polymer system is the so-called test-fluid M1. This polymeric solution is shown to degrade significantly, even for small values of the velocity gradient, as measured by the changes in the macroscopic relaxation time-scales. The second solution is a concentrated polystyrene solution that presents overshoots and undershoots of the polymer conformation dependent of the ratio of vorticity to rate-of-strain. When subjected to large deformations, this polystyrene solution shows not only the possibility of a

  11. Femtosecond laser field induced modifications of electron-transfer processes in Ne{sup +}-He collisions

    SciTech Connect

    Lu Zhenzhong; Chen Deying; Fan Rongwei; Xia Yuanqin

    2012-01-02

    We demonstrate the presence of femtosecond laser induced charge transfer in Ne{sup +}-He collisions. Electron transfer in ion-atom collisions is considerably modified when the collision is embedded in a strong laser field with the laser intensity of {approx}10{sup 15} W/cm{sup 2}. The observed anisotropy of the He{sup +} angular distribution confirms the prediction of early work that the capture probability varies significantly with the laser polarization angle.

  12. Large aperture laser beam alignment system based on far field sampling technique

    NASA Astrophysics Data System (ADS)

    Zhang, J. C.; Liu, D. Z.; Ouyang, X. P.; Kang, J.; Xie, X. L.; Zhou, J.; Gong, L.; Zhu, B. Q.

    2016-11-01

    Laser beam alignment is very important for high-power laser facility. Long laser path and large-aperture lens for alignment are generally used, while the proposed alignment system with a wedge by far-field sampling technique reduces both space and cost requirements. General alignment system for large-aperture laser beam is long in distance and large in volum because of taking near-field sampling technique. With the development of laser fusion facilities, the space for alignment system is limited. A new alignment system for large-aperture laser beam is designed to save space and reduce operating costs. The new alignment for large-aperture laser beam with a wedge is based on far-field sampling technique. The wedge is placed behind the spatial filter to reflect some laser beam as signal light for alignment. Therefore, laser beam diameter in alignment system is small, which can save space for the laser facility. Comparing to general alignment system for large-aperture laser beam, large-aperture lenses for near-field and far-field sampling, long distance laser path are unnecessary for proposed alignment system, which saves cost and space greatly. This alignment system for large-aperture laser beam has been demonstrated well on the Muliti-PW Facility which uses the 7th beam of the SG-Ⅱ Facility as pump source. The experimental results indicate that the average near-field alignment error is less than 1% of reference, and the average far-filed alignment error is less than 5% of spatial filter pinhole diameter, which meet the alignment system requirements for laser beam of Multi-PW Facility.

  13. Dynamics of atoms in strong laser fields I: A quasi analytical model in momentum space based on a Sturmian expansion of the interacting nonlocal Coulomb potential

    NASA Astrophysics Data System (ADS)

    Ongonwou, F.; Tetchou Nganso, H. M.; Ekogo, T. B.; Kwato Njock, M. G.

    2016-12-01

    In this study we present a model that we have formulated in the momentum space to describe atoms interacting with intense laser fields. As a further step, it follows our recent theoretical approach in which the kernel of the reciprocal-space time-dependent Schrödinger equation (TDSE) is replaced by a finite sum of separable potentials, each of them supporting one bound state of atomic hydrogen (Tetchou Nganso et al. 2013). The key point of the model is that the nonlocal interacting Coulomb potential is expanded in a Coulomb Sturmian basis set derived itself from a Sturmian representation of Bessel functions of the first kind in the position space. As a result, this decomposition allows a simple spectral treatment of the TDSE in the momentum space. In order to illustrate the credibility of the model, we have considered the test case of atomic hydrogen driven by a linearly polarized laser pulse, and have evaluated analytically matrix elements of the atomic Hamiltonian and dipole coupling interaction. For various regimes of the laser parameters used in computations our results are in very good agreement with data obtained from other time-dependent calculations.

  14. Information theories for time-dependent harmonic oscillator

    SciTech Connect

    Choi, Jeong Ryeol; Kim, Min-Soo; Kim, Daeyeoul; Maamache, Mustapha; Menouar, Salah; Nahm, In Hyun

    2011-06-15

    Highlights: > Information theories for the general time-dependent harmonic oscillator based on invariant operator method. > Time dependence of entropies and entropic uncertainty relation. > Characteristics of Shannon information and Fisher information. > Application of information theories to particular systems that have time-dependent behavior. - Abstract: Information theories for the general time-dependent harmonic oscillator are described on the basis of invariant operator method. We obtained entropic uncertainty relation of the system and discussed whether it is always larger than or equal to the physically allowed minimum value. Shannon information and Fisher information are derived by means of density operator that satisfies Liouville-von Neumann equation and their characteristics are investigated. Shannon information is independent of time, but Fisher information is explicitly dependent on time as the time functions of the Hamiltonian vary. We can regard that the Fisher information is a local measure since its time behavior is largely affected by local arrangements of the density, whilst the Shannon information plays the role of a global measure of the spreading of density. To promote the understanding, our theory is applied to special systems, the so-called quantum oscillator with time-dependent frequency and strongly pulsating mass system.

  15. Time-dependent stochastic Bethe-Salpeter approach

    NASA Astrophysics Data System (ADS)

    Rabani, Eran; Baer, Roi; Neuhauser, Daniel

    2015-06-01

    A time-dependent formulation for electron-hole excitations in extended finite systems, based on the Bethe-Salpeter equation (BSE), is developed using a stochastic wave function approach. The time-dependent formulation builds on the connection between time-dependent Hartree-Fock (TDHF) theory and the configuration-interaction with single substitution (CIS) method. This results in a time-dependent Schrödinger-like equation for the quasiparticle orbital dynamics based on an effective Hamiltonian containing direct Hartree and screened exchange terms, where screening is described within the random-phase approximation (RPA). To solve for the optical-absorption spectrum, we develop a stochastic formulation in which the quasiparticle orbitals are replaced by stochastic orbitals to evaluate the direct and exchange terms in the Hamiltonian as well as the RPA screening. This leads to an overall quadratic scaling, a significant improvement over the equivalent symplectic eigenvalue representation of the BSE. Application of the time-dependent stochastic BSE (TDsBSE) approach to silicon and CdSe nanocrystals up to size of ≈3000 electrons is presented and discussed.

  16. Watching excitons move: the time-dependent transition density matrix

    NASA Astrophysics Data System (ADS)

    Ullrich, Carsten

    2012-02-01

    Time-dependent density-functional theory allows one to calculate excitation energies and the associated transition densities in principle exactly. The transition density matrix (TDM) provides additional information on electron-hole localization and coherence of specific excitations of the many-body system. We have extended the TDM concept into the real-time domain in order to visualize the excited-state dynamics in conjugated molecules. The time-dependent TDM is defined as an implicit density functional, and can be approximately obtained from the time-dependent Kohn-Sham orbitals. The quality of this approximation is assessed in simple model systems. A computational scheme for real molecular systems is presented: the time-dependent Kohn-Sham equations are solved with the OCTOPUS code and the time-dependent Kohn-Sham TDM is calculated using a spatial partitioning scheme. The method is applied to show in real time how locally created electron-hole pairs spread out over neighboring conjugated molecular chains. The coupling mechanism, electron-hole coherence, and the possibility of charge separation are discussed.

  17. Earthquake Lights: Time-dependent Earth Surface - Ionosphere Coupling Model

    NASA Astrophysics Data System (ADS)

    Pasko, V. P.

    2012-12-01

    Co-seismic luminescence, commonly referred to as Earthquake lights (EQLs), is an atmospheric luminous phenomenon occurring during strong earthquakes and lasting from a fraction of a second to a few minutes [e.g., Derr, J. S., Bull. Seismol. Soc. Am., 63, 2177, 1973; St-Laurent, F., et al., Phys. Chem. Earth, 31, 305, 2006; Herauld and Lira, Nat. Hazards Earth Syst. Sci., 11, 1025, 2011]. Laboratory experiments of Freund, F. T., et al. [JGR, 105, 11001, 2000; JASTP, 71, 1824, 2009, and references therein] demonstrate that rocks subjected to stress force can generate electric currents. During earthquakes these currents can deliver significant amounts of net positive charge to the ground-air interface leading to enhancements in the electric field and corona discharges around ground objects [Freund et al., 2009]. The eyewitness reports [Herauld and Lira, 2011] indicate similarities of the blue glow observed during EQLs to St. Elmo's fire observed during thunderstorms around wing tips of airplanes or around the tall masts of sailing ships [e.g., Wescott, E.M., et al., GRL, 23, 3687, 1996]. Recent work indicates that the vertical currents induced in the stressed rock can map to ionospheric altitudes and create 10s of % variations in the total electron content in the Earth's ionosphere above the earthquake active region [Kuo, C. L., et al., JGR, 116, A10317, 2011]. The magnitudes of the vertical currents estimated by Kuo et al. [2011] based on work by Freund et al. [2009] range from 0.01 to 10 μA/m2. In this talk we report results from a new time-dependent model allowing to calculate currents induced in the ambient atmosphere and corona currents under application of vertical stressed rock currents with arbitrary time variation. We will report test results documenting the model performance under conditions: (1) relaxation toward the classic global electric circuit conditions in fair weather regions when ionosphere is maintained at 300 kV with respect to the ground; (2

  18. Time-dependent quantum wave packet dynamics to study charge transfer in heavy particle collisions

    NASA Astrophysics Data System (ADS)

    Zhang, Song Bin; Wu, Yong; Wang, Jian Guo

    2016-12-01

    The method of time-dependent quantum wave packet dynamics has been successfully extended to study the charge transfer/exchange process in low energy two-body heavy particle collisions. The collision process is described by coupled-channel equations with diabatic potentials and (radial and rotational) couplings. The time-dependent coupled equations are propagated with the multiconfiguration time-dependent Hartree method and the modulo squares of S-matrix is extracted from the wave packet by the flux operator with complex absorbing potential (FCAP) method. The calculations of the charge transfer process 12Σ+ H-(1s2) +Li(1 s22 s ) →22Σ+ /32 Σ+ /12 Π H(1 s ) +Li-(1s 22 s 2 l ) (l =s ,p ) at the incident energy of about [0.3, 1.3] eV are illustrated as an example. It shows that the calculated reaction probabilities by the present FCAP reproduce that of quantum-mechanical molecular-orbital close-coupling very well, including the peak structures contributed by the resonances. Since time-dependent external interactions can be directly included in the present FCAP calculations, the successful implementation of FCAP provides us a powerful potential tool to study the quantum control of heavy particle collisions by lasers in the near future.

  19. Time-dependent density functional theory for quantum transport.

    PubMed

    Zheng, Xiao; Chen, GuanHua; Mo, Yan; Koo, SiuKong; Tian, Heng; Yam, ChiYung; Yan, YiJing

    2010-09-21

    Based on our earlier works [X. Zheng et al., Phys. Rev. B 75, 195127 (2007); J. S. Jin et al., J. Chem. Phys. 128, 234703 (2008)], we propose a rigorous and numerically convenient approach to simulate time-dependent quantum transport from first-principles. The proposed approach combines time-dependent density functional theory with quantum dissipation theory, and results in a useful tool for studying transient dynamics of electronic systems. Within the proposed exact theoretical framework, we construct a number of practical schemes for simulating realistic systems such as nanoscopic electronic devices. Computational cost of each scheme is analyzed, with the expected level of accuracy discussed. As a demonstration, a simulation based on the adiabatic wide-band limit approximation scheme is carried out to characterize the transient current response of a carbon nanotube based electronic device under time-dependent external voltages.

  20. Full-counting statistics of time-dependent conductors

    NASA Astrophysics Data System (ADS)

    Benito, Mónica; Niklas, Michael; Kohler, Sigmund

    2016-11-01

    We develop a scheme for the computation of the full-counting statistics of transport described by Markovian master equations with an arbitrary time dependence. It is based on a hierarchy of generalized density operators, where the trace of each operator yields one cumulant. This direct relation offers a better numerical efficiency than the equivalent number-resolved master equation. The proposed method is particularly useful for conductors with an elaborate time dependence stemming, e.g., from pulses or combinations of slow and fast parameter switching. As a test bench for the evaluation of the numerical stability, we consider time-independent problems for which the full-counting statistics can be computed by other means. As applications, we study cumulants of higher order for two time-dependent transport problems of recent interest, namely steady-state coherent transfer by adiabatic passage (CTAP) and Landau-Zener-Stückelberg-Majorana (LZSM) interference in an open double quantum dot.

  1. Control of focusing fields for positron acceleration in nonlinear plasma wakes using multiple laser modes

    SciTech Connect

    Yu, L.-L. Li, F.-Y.; Chen, M.; Weng, S.-M.; Schroeder, C. B.; Benedetti, C.; Esarey, E.; Sheng, Z.-M.

    2014-12-15

    Control of transverse wakefields in the nonlinear laser-driven bubble regime using a combination of Hermite-Gaussian laser modes is proposed. By controlling the relative intensity ratio of the two laser modes, the focusing force can be controlled, enabling matched beam propagation for emittance preservation. A ring bubble can be generated with a large longitudinal accelerating field and a transverse focusing field suitable for positron beam focusing and acceleration.

  2. Laser Light-field Fusion for Wide-field Lensfree On-chip Phase Contrast Microscopy of Nanoparticles

    PubMed Central

    Kazemzadeh, Farnoud; Wong, Alexander

    2016-01-01

    Wide-field lensfree on-chip microscopy, which leverages holography principles to capture interferometric light-field encodings without lenses, is an emerging imaging modality with widespread interest given the large field-of-view compared to lens-based techniques. In this study, we introduce the idea of laser light-field fusion for lensfree on-chip phase contrast microscopy for detecting nanoparticles, where interferometric laser light-field encodings acquired using a lensfree, on-chip setup with laser pulsations at different wavelengths are fused to produce marker-free phase contrast images of particles at the nanometer scale. As a proof of concept, we demonstrate, for the first time, a wide-field lensfree on-chip instrument successfully detecting 300 nm particles across a large field-of-view of ~30 mm2 without any specialized or intricate sample preparation, or the use of synthetic aperture- or shift-based techniques. PMID:27958348

  3. Laser Light-field Fusion for Wide-field Lensfree On-chip Phase Contrast Microscopy of Nanoparticles

    NASA Astrophysics Data System (ADS)

    Kazemzadeh, Farnoud; Wong, Alexander

    2016-12-01

    Wide-field lensfree on-chip microscopy, which leverages holography principles to capture interferometric light-field encodings without lenses, is an emerging imaging modality with widespread interest given the large field-of-view compared to lens-based techniques. In this study, we introduce the idea of laser light-field fusion for lensfree on-chip phase contrast microscopy for detecting nanoparticles, where interferometric laser light-field encodings acquired using a lensfree, on-chip setup with laser pulsations at different wavelengths are fused to produce marker-free phase contrast images of particles at the nanometer scale. As a proof of concept, we demonstrate, for the first time, a wide-field lensfree on-chip instrument successfully detecting 300 nm particles across a large field-of-view of ~30 mm2 without any specialized or intricate sample preparation, or the use of synthetic aperture- or shift-based techniques.

  4. Laser Light-field Fusion for Wide-field Lensfree On-chip Phase Contrast Microscopy of Nanoparticles.

    PubMed

    Kazemzadeh, Farnoud; Wong, Alexander

    2016-12-13

    Wide-field lensfree on-chip microscopy, which leverages holography principles to capture interferometric light-field encodings without lenses, is an emerging imaging modality with widespread interest given the large field-of-view compared to lens-based techniques. In this study, we introduce the idea of laser light-field fusion for lensfree on-chip phase contrast microscopy for detecting nanoparticles, where interferometric laser light-field encodings acquired using a lensfree, on-chip setup with laser pulsations at different wavelengths are fused to produce marker-free phase contrast images of particles at the nanometer scale. As a proof of concept, we demonstrate, for the first time, a wide-field lensfree on-chip instrument successfully detecting 300 nm particles across a large field-of-view of ~30 mm(2) without any specialized or intricate sample preparation, or the use of synthetic aperture- or shift-based techniques.

  5. Parametric distortion of the optical absorption edge of a magnetic semiconductor by a strong laser field

    SciTech Connect

    Nunes, O.A.C.

    1985-09-15

    The influence of a strong laser field on the optical absorption edge of a direct-gap magnetic semiconductor is considered. It is shown that as the strong laser intensity increases the absorption coefficient is modified so as to give rise to an absorption tail below the free-field forbidden gap. An application is made for the case of the EuO.

  6. Time-dependent perturbation theory for inelastic scattering

    NASA Astrophysics Data System (ADS)

    Cross, R. J.

    1982-08-01

    We show by numerical integration that the first-order, time-dependent, Magnus approximation agrees with the first-order, exponential, distorted-wave approximation to within a few percent, provided that the trajectory used for the time-dependent calculation is characterized by the arithmetic mean of the initial and final velocities and the arithmetic mean of the initial and final orbital angular momenta. Calculations are done for rotational energy transfer from an exponentially repulsive potential characteristic of He+H2 and for a Lennard-Jones potential characteristic of Ar+N2.

  7. Time-dependent Bragg diffraction by multilayer gratings

    NASA Astrophysics Data System (ADS)

    André, Jean-Michel; Jonnard, Philippe

    2016-01-01

    Time-dependent Bragg diffraction by multilayer gratings working by reflection or by transmission is investigated. The study is performed by generalizing the time-dependent coupled-wave theory previously developed for one-dimensional photonic crystals (André J-M and Jonnard P 2015 J. Opt. 17 085609) and also by extending the Takagi-Taupin approach of the dynamical theory of diffraction. The indicial response is calculated. It presents a time delay with a transient time that is a function of the extinction length for reflection geometry and of the extinction length combined with the thickness of the grating for transmission geometry.

  8. Enhanced thermopower under a time-dependent gate voltage

    NASA Astrophysics Data System (ADS)

    Crépieux, Adeline; Šimkovic, Fedor; Cambon, Benjamin; Michelini, Fabienne

    2011-04-01

    We derive formal expressions of time-dependent energy and heat currents through a nanoscopic device using the Keldysh nonequilibrium Green function technique. Numerical results are reported for a metal-dot-metal junction where the dot level energy is abruptly changed by a step-shaped voltage pulse. Analytical linear responses are obtained for the time-dependent thermoelectric coefficients. We show that in the transient regime the Seebeck coefficient can be enhanced by an amount (as much as 40%) controlled by both the dot energy and the height of the voltage step.

  9. Two-stream instability with time-dependent drift velocity

    DOE PAGES

    Qin, Hong; Davidson, Ronald C.

    2014-06-26

    The classical two-stream instability driven by a constant relative drift velocity between two plasma components is extended to the case with time-dependent drift velocity. A solution method is developed to rigorously define and calculate the instability growth rate for linear perturbations relative to the time-dependent unperturbed two-stream motions. The stability diagrams for the oscillating two-stream instability are presented over a large region of parameter space. It is shown that the growth rate for the classical two-stream instability can be significantly reduced by adding an oscillatory component to the relative drift velocity.

  10. Choice of Variables and Preconditioning for Time Dependent Problems

    NASA Technical Reports Server (NTRS)

    Turkel, Eli; Vatsa, Verr N.

    2003-01-01

    We consider the use of low speed preconditioning for time dependent problems. These are solved using a dual time step approach. We consider the effect of this dual time step on the parameter of the low speed preconditioning. In addition, we compare the use of two sets of variables, conservation and primitive variables, to solve the system. We show the effect of these choices on both the convergence to a steady state and the accuracy of the numerical solutions for low Mach number steady state and time dependent flows.

  11. Directional solidification of a planar interface in the presence of a time-dependent electric current

    NASA Technical Reports Server (NTRS)

    Brush, L. N.; Coriell, S. R.; Mcfadden, G. B.

    1990-01-01

    Directional solidification of pure materials and binary alloys with a planar crystal-metal interface in the presence of a time-dependent electric current is considered. For a variety of time-dependent currents, the temperature fields and the interface velocity as functions of time are presented for indium antimonide and bismuth and for the binary alloys germanium-gallium and tin-bismuth. For the alloys, the solid composition is calculated as a function of position. Quantitative predictions are made of the effect of an electrical pulse on the solute distribution in the solidified material.

  12. Ion-implantation effect on time-dependent breakdown in SiO2

    NASA Technical Reports Server (NTRS)

    Li, S. P.

    1975-01-01

    It was experimentally demonstrated that the field emission of positive ions from the metal SiO2 interface in MOS structures can be controlled by introducing a positive charge in a small ion-implantation dose to a shallow depth below the metal electrode. Considerable improvement of time-dependent breakdown was noted in structures implanted in this manner as opposed to nonimplanted ones. This experiment confirms the model proposed by Li and Maserjian (1975) for radiation effect on time-dependent breakdown.

  13. A new concept in laser-assisted chemistry - The electronic-field representation

    NASA Technical Reports Server (NTRS)

    George, T. F.; Zimmerman, I. H.; Yuan, J.-M.; Laing, J. R.; Devries, P. L.

    1977-01-01

    Electronic-field representation is proposed as a technique for laser-assisted chemistry. Specifically, it is shown that several field-assisted chemical processes can be described in terms of mixed matter-field quantum states and their associated energies. The technique may be used to analyze the effects exerted by an intense laser on both bound and unbound molecular systems, and to investigate other field-induced effects including multiphoton processes, emission, and photodissociation.

  14. A 7 T Pulsed Magnetic Field Generator for Magnetized Laser Plasma Experiments

    NASA Astrophysics Data System (ADS)

    Hu, Guangyue; Liang, Yihan; Song, Falun; Yuan, Peng; Wang, Yulin; Zhao, Bin; Zheng, Jian

    2015-02-01

    A pulsed magnetic field generator was developed to study the effect of a magnetic field on the evolution of a laser-generated plasma. A 40 kV pulsed power system delivered a fast (~230 ns), 55 kA current pulse into a single-turn coil surrounding the laser target, using a capacitor bank of 200 nF, a laser-triggered switch and a low-impedance strip transmission line. A one-dimensional uniform 7 T pulsed magnetic field was created using a Helmholtz coil pair with a 6 mm diameter. The pulsed magnetic field was controlled to take effect synchronously with a nanosecond heating laser beam, a femtosecond probing laser beam and an optical Intensified Charge Coupled Device (ICCD) detector. The preliminary experiments demonstrate bifurcation and focusing of plasma expansion in a transverse magnetic field.

  15. Time dependent pre-treatment EPID dosimetry for standard and FFF VMAT.

    PubMed

    Podesta, Mark; Nijsten, Sebastiaan M J J G; Persoon, Lucas C G G; Scheib, Stefan G; Baltes, Christof; Verhaegen, Frank

    2014-08-21

    Methods to calibrate Megavoltage electronic portal imaging devices (EPIDs) for dosimetry have been previously documented for dynamic treatments such as intensity modulated radiotherapy (IMRT) using flattened beams and typically using integrated fields. While these methods verify the accumulated field shape and dose, the dose rate and differential fields remain unverified. The aim of this work is to provide an accurate calibration model for time dependent pre-treatment dose verification using amorphous silicon (a-Si) EPIDs in volumetric modulated arc therapy (VMAT) for both flattened and flattening filter free (FFF) beams. A general calibration model was created using a Varian TrueBeam accelerator, equipped with an aS1000 EPID, for each photon spectrum 6 MV, 10 MV, 6 MV-FFF, 10 MV-FFF. As planned VMAT treatments use control points (CPs) for optimization, measured images are separated into corresponding time intervals for direct comparison with predictions. The accuracy of the calibration model was determined for a range of treatment conditions. Measured and predicted CP dose images were compared using a time dependent gamma evaluation using criteria (3%, 3 mm, 0.5 sec). Time dependent pre-treatment dose verification is possible without an additional measurement device or phantom, using the on-board EPID. Sufficient data is present in trajectory log files and EPID frame headers to reliably synchronize and resample portal images. For the VMAT plans tested, significantly more deviation is observed when analysed in a time dependent manner for FFF and non-FFF plans than when analysed using only the integrated field. We show EPID-based pre-treatment dose verification can be performed on a CP basis for VMAT plans. This model can measure pre-treatment doses for both flattened and unflattened beams in a time dependent manner which highlights deviations that are missed in integrated field verifications.

  16. Simulations of time-dependent drive asymmetries for shock ignition

    NASA Astrophysics Data System (ADS)

    Loomis, Eric; Dodd, Evan; Cobble, James; Marinak, Marty; Sauppe, Joshua

    2016-10-01

    Shock Ignition (SI) is an extension of conventional inertial confinement fusion (ICF) where a strong shock heats low temperature, but highly compressed, deuterium-tritium fuel to ignition conditions. The conditions for maximum pressure amplification by the ignitor shock have been predicted in one-dimensional geometry where shock heating is most efficient. In real experiments, asymmetries in the flow field almost always take on 2- and 3-dimensional structure. To study the degradation in heating efficiency of the ignitor shock when interacting with asymmetric rebounding shocks and multi-dimensional flow we have performed a series of HYDRA simulations that use the indirect drive high foot design of Dittrich et al.. In our simulations we truncated the radiation drive to peak at 270 eV and used the remaining energy to directly irradiate the capsule with a spherical laser source to create the ignitor shock. Legendre mode asymmetries were applied to the radiation field at different times during implosion of the capsule producing fuel and rebounding shock asymmetries that significantly reduced the ignitor efficiency. We will present how the heating is reduced for asymmetries in the pulse foot and peak.

  17. Numerical Density-to-Potential Inversions in Time-dependent Density Functional Theory

    NASA Astrophysics Data System (ADS)

    Jensen, Daniel; Inchaustegui, Jean Pierre; Wasserman, Adam

    2014-03-01

    Time-dependent Density Functional Theory (TDDFT) is a formally exact method for solving the quantum many-body problem. In Kohn-Sham TDDFT, a fictitious noninteracting system is defined that exactly reproduces the time-dependent density of the interacting system. The potential that determines this noninteracting system (the time-dependent Kohn-Sham potential) has been proven to exist under certain restrictions, but finding the exact Kohn-Sham potential for a given density remains challenging. We show that this ill-posed inverse problem requires some form of regularization to produce realistic Kohn-Sham potentials. We explore various forms of regularization and illustrate how they work on simple one-dimensional model systems. We also show how our method can be applied to problems with both particle-in-a-box and periodic boundary conditions subject to oscillating electric fields.

  18. CONDENSED MATTER: ELECTRONICSTRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICALPROPERTIES: Time-Dependent Transport in Nanoscale Devices

    NASA Astrophysics Data System (ADS)

    Chen, Zhi-Dong; Zhang, Jin-Yu; Yu, Zhi-Ping

    2009-03-01

    A method for simulating ballistic time-dependent device transport, which solves the time-dependent Schrödinger equation using the finite difference time domain (FDTD) method together with Poisson's equation, is described in detail. The effective mass Schrödinger equation is solved. The continuous energy spectrum of the system is discretized using adaptive mesh, resulting in energy levels that sample the density-of-states. By calculating time evolution of wavefunctions at sampled energies, time-dependent transport characteristics such as current and charge density distributions are obtained. Simulation results in a nanowire and a coaxially gated carbon nanotube field-effect transistor (CNTFET) are presented. Transient effects, e.g., finite rising time, are investigated in these devices.

  19. Laser field induced optical gain in a group III-V quantum wire

    NASA Astrophysics Data System (ADS)

    Saravanan, Subramanian; Peter, Amalorpavam John; Lee, Chang Woo

    2016-08-01

    Effect of intense high frequency laser field on the electronic and optical properties of heavy hole exciton in an InAsP/InP quantum well wire is investigated taking into consideration of the spatial confinement. Laser field induced exciton binding energies, optical band gap, oscillator strength and the optical gain in the InAs0.8P0.2/InP quantum well wire are studied. The variational formulism is applied to find the respective energies. The laser field induced optical properties are studied. The optical gain as a function of photon energy, in the InAs0.8P0.2/InP quantum wire, is obtained in the presence of intense laser field. The compact density matrix method is employed to obtain the optical gain. The results show that the 1.55 μm wavelength for the fibre optic telecommunication applications is achieved for 45 Å wire radius in the absence of laser field intensity whereas the 1.55 μm wavelength is obtained for 40 Å if the amplitude of the laser field amplitude parameter is 50 Å. The characterizing wavelength for telecommunication network is optimized when the intense laser field is applied for the system. It is hoped that the obtained optical gain in the group III-V narrow quantum wire can be applied for fabricating laser sources for achieving the preferred telecommunication wavelength.

  20. Simulation of Temperature Field Distribution for Cutting the Temperated Glass by Ultraviolet Laser

    NASA Astrophysics Data System (ADS)

    Yang, B. J.; He, Y. C.; Dai, F.; Lin, X. C.

    2017-03-01

    The finite element software ANSYS was adopted to simulate the temperature field distribution for laser cutting tempered glass, and the influence of different process parameters, including laser power, glass thickness and cutting speed, on temperature field distribution was studied in detail. The results show that the laser power has a greater influence on temperature field distribution than other paremeters, and when the laser power gets to 60W, the highest temperature reaches 749°C, which is higher than the glass softening temperature. It reflects the material near the laser spot is melted and the molten slag is removed by the high-energy water beam quickly. Finally, through the water guided laser cutting tempered glass experiment the FEM theoretical analysis was verified.

  1. Phase space theory of Bose-Einstein condensates and time-dependent modes

    SciTech Connect

    Dalton, B.J.

    2012-10-15

    A phase space theory approach for treating dynamical behaviour of Bose-Einstein condensates applicable to situations such as interferometry with BEC in time-dependent double well potentials is presented. Time-dependent mode functions are used, chosen so that one, two, Horizontal-Ellipsis highly occupied modes describe well the physics of interacting condensate bosons in time dependent potentials at well below the transition temperature. Time dependent mode annihilation, creation operators are represented by time dependent phase variables, but time independent total field annihilation, creation operators are represented by time independent field functions. Two situations are treated, one (mode theory) is where specific mode annihilation, creation operators and their related phase variables and distribution functions are dealt with, the other (field theory) is where only field creation, annihilation operators and their related field functions and distribution functionals are involved. The field theory treatment is more suitable when large boson numbers are involved. The paper focuses on the hybrid approach, where the modes are divided up between condensate (highly occupied) modes and non-condensate (sparsely occupied) modes. It is found that there are extra terms in the Ito stochastic equations both for the stochastic phases and stochastic fields, involving coupling coefficients defined via overlap integrals between mode functions and their time derivatives. For the hybrid approach both the Fokker-Planck and functional Fokker-Planck equations differ from those derived via the correspondence rules, the drift vectors are unchanged but the diffusion matrices contain additional terms involving the coupling coefficients. Results are also presented for the combined approach where all the modes are treated as one set. Here both the Fokker-Planck and functional Fokker-Planck equations are exactly the same as those derived via the correspondence rules. However, although the

  2. Adjoint-Based Methodology for Time-Dependent Optimization

    NASA Technical Reports Server (NTRS)

    Yamaleev, N. K.; Diskin, B.; Nielsen, E. J.

    2008-01-01

    This paper presents a discrete adjoint method for a broad class of time-dependent optimization problems. The time-dependent adjoint equations are derived in terms of the discrete residual of an arbitrary finite volume scheme which approximates unsteady conservation law equations. Although only the 2-D unsteady Euler equations are considered in the present analysis, this time-dependent adjoint method is applicable to the 3-D unsteady Reynolds-averaged Navier-Stokes equations with minor modifications. The discrete adjoint operators involving the derivatives of the discrete residual and the cost functional with respect to the flow variables are computed using a complex-variable approach, which provides discrete consistency and drastically reduces the implementation and debugging cycle. The implementation of the time-dependent adjoint method is validated by comparing the sensitivity derivative with that obtained by forward mode differentiation. Our numerical results show that O(10) optimization iterations of the steepest descent method are needed to reduce the objective functional by 3-6 orders of magnitude for test problems considered.

  3. Stability on time-dependent domains: convective and dilution effects

    NASA Astrophysics Data System (ADS)

    Krechetnikov, R.; Knobloch, E.

    2017-03-01

    We explore near-critical behavior of spatially extended systems on time-dependent spatial domains with convective and dilution effects due to domain flow. As a paradigm, we use the Swift-Hohenberg equation, which is the simplest nonlinear model with a non-zero critical wavenumber, to study dynamic pattern formation on time-dependent domains. A universal amplitude equation governing weakly nonlinear evolution of patterns on time-dependent domains is derived and proves to be a generalization of the standard Ginzburg-Landau equation. Its key solutions identified here demonstrate a substantial variety-spatially periodic states with a time-dependent wavenumber, steady spatially non-periodic states, and pulse-train solutions-in contrast to extended systems on time-fixed domains. The effects of domain flow, such as bifurcation delay due to domain growth and destabilization due to oscillatory domain flow, on the Eckhaus instability responsible for phase slips in spatially periodic states are analyzed with the help of both local and global stability analyses. A nonlinear phase equation describing the approach to a phase-slip event is derived. Detailed analysis of a phase slip using multiple time scale methods demonstrates different mechanisms governing the wavelength changing process at different stages.

  4. Time dependent solution for acceleration of tau-leaping

    SciTech Connect

    Fu, Jin; Wu, Sheng; Petzold, Linda R.

    2013-02-15

    The tau-leaping method is often effective for speeding up discrete stochastic simulation of chemically reacting systems. However, when fast reactions are involved, the speed-up for this method can be quite limited. One way to address this is to apply a stochastic quasi-steady state assumption. However we must be careful when using this assumption. If the fast subsystem cannot reach a steady distribution fast enough, the quasi-steady-state assumption will propagate error into the simulation. To avoid these errors, we propose to use the time dependent solution rather than the quasi-steady-state. Generally speaking, the time dependent solution is not easy to derive for an arbitrary network. However, for some common motifs we do have time dependent solutions. We derive the time dependent solutions for these motifs, and then show how they can be used with tau-leaping to achieve substantial speed-ups, including for a realistic model of blood coagulation. Although the method is complicated, we have automated it.

  5. Student Understanding of Time Dependence in Quantum Mechanics

    ERIC Educational Resources Information Center

    Emigh, Paul J.; Passante, Gina; Shaffer, Peter S.

    2015-01-01

    The time evolution of quantum states is arguably one of the more difficult ideas in quantum mechanics. In this article, we report on results from an investigation of student understanding of this topic after lecture instruction. We demonstrate specific problems that students have in applying time dependence to quantum systems and in recognizing…

  6. Shoulder pain and time dependent structure in wheelchair propulsion variability.

    PubMed

    Jayaraman, Chandrasekaran; Moon, Yaejin; Sosnoff, Jacob J

    2016-07-01

    Manual wheelchair propulsion places considerable repetitive mechanical strain on the upper limbs leading to shoulder injury and pain. While recent research indicates that the amount of variability in wheelchair propulsion and shoulder pain may be related. There has been minimal inquiry into the fluctuation over time (i.e. time-dependent structure) in wheelchair propulsion variability. Consequently the purpose of this investigation was to examine if the time-dependent structure in the wheelchair propulsion parameters are related to shoulder pain. 27 experienced wheelchair users manually propelled their own wheelchair fitted with a SMARTWheel on a roller at 1.1m/s for 3min. Time-dependent structure of cycle-to-cycle fluctuations in contact angle and inter push time interval was quantified using sample entropy (SampEn) and compared between the groups with/without shoulder pain using non-parametric statistics. Overall findings were, (1) variability observed in contact angle fluctuations during manual wheelchair propulsion is structured (Z=3.15;p<0.05), (2) individuals with shoulder pain exhibited higher SampEn magnitude for contact angle during wheelchair propulsion than those without pain (χ(2)(1)=6.12;p<0.05); and (3) SampEn of contact angle correlated significantly with self-reported shoulder pain (rs (WUSPI) =0.41;rs (VAS)=0.56;p<0.05). It was concluded that the time-dependent structure in wheelchair propulsion may provide novel information for tracking and monitoring shoulder pain.

  7. Time dependent solution for acceleration of tau-leaping

    NASA Astrophysics Data System (ADS)

    Fu, Jin; Wu, Sheng; Petzold, Linda R.

    2013-02-01

    The tau-leaping method is often effective for speeding up discrete stochastic simulation of chemically reacting systems. However, when fast reactions are involved, the speed-up for this method can be quite limited. One way to address this is to apply a stochastic quasi-steady state assumption. However we must be careful when using this assumption. If the fast subsystem cannot reach a steady distribution fast enough, the quasi-steady-state assumption will propagate error into the simulation. To avoid these errors, we propose to use the time dependent solution rather than the quasi-steady-state. Generally speaking, the time dependent solution is not easy to derive for an arbitrary network. However, for some common motifs we do have time dependent solutions. We derive the time dependent solutions for these motifs, and then show how they can be used with tau-leaping to achieve substantial speed-ups, including for a realistic model of blood coagulation. Although the method is complicated, we have automated it.

  8. Controlling Nonsequential Double Ionization in Two-Color Circularly Polarized Femtosecond Laser Fields

    NASA Astrophysics Data System (ADS)

    Mancuso, Christopher A.; Dorney, Kevin M.; Hickstein, Daniel D.; Chaloupka, Jan L.; Ellis, Jennifer L.; Dollar, Franklin J.; Knut, Ronny; Grychtol, Patrik; Zusin, Dmitriy; Gentry, Christian; Gopalakrishnan, Maithreyi; Kapteyn, Henry C.; Murnane, Margaret M.

    2016-09-01

    Atoms undergoing strong-field ionization in two-color circularly polarized femtosecond laser fields exhibit unique two-dimensional photoelectron trajectories and can emit bright circularly polarized extreme ultraviolet and soft-x-ray beams. In this Letter, we present the first experimental observation of nonsequential double ionization in these tailored laser fields. Moreover, we can enhance or suppress nonsequential double ionization by changing the intensity ratio and helicity of the two driving laser fields to maximize or minimize high-energy electron-ion rescattering. Our experimental results are explained through classical simulations, which also provide insight into how to optimize the generation of circularly polarized high harmonic beams.

  9. Fast magnetic field annihilation driven by two laser pulses in underdense plasma

    SciTech Connect

    Gu, Y. J.; Kumar, D.; Weber, S.; Korn, G.; Klimo, O.; Bulanov, S. V.; Esirkepov, T. Zh.

    2015-10-15

    Fast magnetic annihilation is investigated by using 2.5-dimensional particle-in-cell simulations of two parallel ultra-short petawatt laser pulses co-propagating in underdense plasma. The magnetic field generated by the laser pulses annihilates in a current sheet formed between the pulses. Magnetic field energy is converted to an inductive longitudinal electric field, which efficiently accelerates the electrons of the current sheet. This new regime of collisionless relativistic magnetic field annihilation with a timescale of tens of femtoseconds can be extended to near-critical and overdense plasma with the ultra-high intensity femtosecond laser pulses.

  10. LETTER TO THE EDITOR: H2+ in intense laser field pulses: ionization versus dissociation within moving nucleus simulations

    NASA Astrophysics Data System (ADS)

    Rotenberg, Benjamin; Taïeb, Richard; Véniard, Valérie; Maquet, Alfred

    2002-09-01

    The theory of the interaction of the H2+ molecular ion with an intense short laser pulse is modelled by solving the time-dependent Schrödinger equation for the electronic degree of freedom while the nuclear motion is described classically. This method allows us to discuss the influence of the pulse duration on the respective weights of ionization and dissociation.

  11. Intensity dependence of the H{sub 2}{sup +} ionization rates in Ti:sapphire laser fields above the Coulomb-explosion threshold

    SciTech Connect

    Sabzyan, Hassan; Vafaee, Mohsen

    2005-06-15

    Ionization rates of the hydrogen molecular ion H{sub 2}{sup +} under linearly polarized pulse of intense laser fields are simulated by direct solution of the fixed-nuclei time-dependent Schroedinger equation for the Ti:sapphire laser lines {lambda}=790 and 800 nm at high intensities starting from just above the Coulomb explosion threshold (i.e., 6.0x10{sup 13}, 1.0x10{sup 14}, 3.2x10{sup 14}, and 1.4x10{sup 15} W cm{sup -2}). Results obtained in this research exhibit a high degree of complexity for the R-dependent enhanced ionization rates for the H{sub 2}{sup +} system in these intense laser fields. The R-dependent ionization peaks move towards small internuclear distances and their structure becomes simpler and smoother with the increase in the intensity of the laser pulse, i.e., with the decrease in the Keldysh parameter. Results obtained in this research are comparable to and even more reliable than the results of other theoretical calculations reported recently and successfully simulate the experimental ionization data.

  12. Explosions of water clusters in intense laser fields

    SciTech Connect

    Kumarappan, V.; Krishnamurthy, M.; Mathur, D.

    2003-06-01

    Energetic, highly charged oxygen ions O{sup q+} (q{<=}6), are copiously produced upon laser field-induced disassembly of highly charged water clusters, (H{sub 2}O){sub n} and (D{sub 2}O){sub n}, n{approx}60, that are formed by seeding high-pressure helium or argon with water vapor. Ar{sub n} clusters (n{approx}40 000) formed under similar experimental conditions are found to undergo disassembly in the Coulomb explosion regime, with the energies of Ar{sup q+} ions showing a q{sup 2} dependence. Water clusters, which are argued to be considerably smaller in size, should also disassemble in the same regime, but the energies of fragment O{sup q+} ions are found to depend linearly on q which, according to prevailing wisdom, ought to be a signature of hydrodynamic expansion that is expected of much larger clusters. The implication of these observations on our understanding of the two cluster explosion regimes, Coulomb explosion and hydrodynamic expansion, is discussed. Our results indicate that charge state dependences of ion energy do not constitute an unambiguous experimental signature of cluster explosion regime.

  13. Using Multiple Whole-Cell Recordings to Study Spike-Timing-Dependent Plasticity in Acute Neocortical Slices

    PubMed Central

    Lalanne, Txomin; Abrahamsson, Therese; Sjöström, P. Jesper

    2017-01-01

    This protocol provides a method for quadruple whole-cell recording to study synaptic plasticity of neocortical connections, with a special focus on spike-timing-dependent plasticity (STDP). It also describes how to morphologically identify recorded cells from two-photon laser-scanning microscopy (2PLSM) stacks. PMID:27250948

  14. TOPICAL REVIEW: The Bloch wave operator: generalizations and applications: II. The time-dependent case

    NASA Astrophysics Data System (ADS)

    Jolicard, Georges; Killingbeck, John P.

    2003-10-01

    Part II of the review shows how the stationary Bloch wave operator of part I can be suitably modified to give a time-dependent wave operator. This operator makes it possible to use a relatively small active space in order to describe the dynamical processes which occur in quantum mechanical systems which have a time-dependent Hamiltonian. A close study is made of the links between the time-dependent and time-independent wave operators at the adiabatic limit; the analysis clarifies the way in which the wave operator formalism allows the time evolution of a system or a wave packet to be described in terms of a fast evolution inside the active space together with weak transitions out of this space which can be treated by perturbation methods. Two alternative wave operator equations of motion are derived and analysed. The first one is a non-linear differential equation in the usual Hilbert space; the second one is a differential equation in an extended Hilbert space with an extra time variable added and becomes equivalent to the usual Bloch equation when the Floquet Hamiltonian is taken in place of the ordinary Hamiltonian. A study is made of the close relationships between the time-dependent wave operator formalism, the Floquet theory and the (t, t') theory. Some original methods of solution of the two forms of wave operator equation are proposed and lead to new techniques of integration for the time-dependent Schrödinger equation (e.g., the generalized Green equation procedure). Mixed procedures involving both the time-independent and time-dependent wave operators are shown to be applicable to the internal eigenstate problem for large complex matrices. A detailed account is given of the description of inelastic and photoreactive processes by means of the time-dependent wave operator formalism, with particular attention to laser-molecule interactions. The emphasis is on projection operator techniques, with special attention being given to the method of selection of

  15. Optimal adaptive control for quantum metrology with time-dependent Hamiltonians

    NASA Astrophysics Data System (ADS)

    Pang, Shengshi; Jordan, Andrew N.

    2017-03-01

    Quantum metrology has been studied for a wide range of systems with time-independent Hamiltonians. For systems with time-dependent Hamiltonians, however, due to the complexity of dynamics, little has been known about quantum metrology. Here we investigate quantum metrology with time-dependent Hamiltonians to bridge this gap. We obtain the optimal quantum Fisher information for parameters in time-dependent Hamiltonians, and show proper Hamiltonian control is generally necessary to optimize the Fisher information. We derive the optimal Hamiltonian control, which is generally adaptive, and the measurement scheme to attain the optimal Fisher information. In a minimal example of a qubit in a rotating magnetic field, we find a surprising result that the fundamental limit of T2 time scaling of quantum Fisher information can be broken with time-dependent Hamiltonians, which reaches T4 in estimating the rotation frequency of the field. We conclude by considering level crossings in the derivatives of the Hamiltonians, and point out additional control is necessary for that case.

  16. Optimal adaptive control for quantum metrology with time-dependent Hamiltonians.

    PubMed

    Pang, Shengshi; Jordan, Andrew N

    2017-03-09

    Quantum metrology has been studied for a wide range of systems with time-independent Hamiltonians. For systems with time-dependent Hamiltonians, however, due to the complexity of dynamics, little has been known about quantum metrology. Here we investigate quantum metrology with time-dependent Hamiltonians to bridge this gap. We obtain the optimal quantum Fisher information for parameters in time-dependent Hamiltonians, and show proper Hamiltonian control is generally necessary to optimize the Fisher information. We derive the optimal Hamiltonian control, which is generally adaptive, and the measurement scheme to attain the optimal Fisher information. In a minimal example of a qubit in a rotating magnetic field, we find a surprising result that the fundamental limit of T(2) time scaling of quantum Fisher information can be broken with time-dependent Hamiltonians, which reaches T(4) in estimating the rotation frequency of the field. We conclude by considering level crossings in the derivatives of the Hamiltonians, and point out additional control is necessary for that case.

  17. Time-dependent ionization balance model for non-LTE plasma

    SciTech Connect

    Lee, Y.T.; Zimmerman, G.B.; Bailey, D.S.; Dickson, D.; Kim, D.

    1986-05-07

    We have developed a detailed configuration-accounting kinetic model for calculating time-dependent ionization-balance and ion-level populations in non-local thermal-equilibrium (non-LTE) plasmas. We use these population estimates in computing spectral line intensities, line ratios, and synthetic spectra, and in fitting these calculated values to experimental measurements. The model is also used to design laboratory x-ray laser experiments. For this purpose, it is self-consistently coupled to the hydrodynamics code LASNEX. 20 refs., 14 figs.

  18. Wide-Field Optic for Autonomous Acquisition of Laser Link

    NASA Technical Reports Server (NTRS)

    Page, Norman A.; Charles, Jeffrey R.; Biswas, Abhijit

    2011-01-01

    An innovation reported in Two-Camera Acquisition and Tracking of a Flying Target, NASA Tech Briefs, Vol. 32, No. 8 (August 2008), p. 20, used a commercial fish-eye lens and an electronic imaging camera for initially locating objects with subsequent handover to an actuated narrow-field camera. But this operated against a dark-sky background. An improved solution involves an optical design based on custom optical components for the wide-field optical system that directly addresses the key limitations in acquiring a laser signal from a moving source such as an aircraft or a spacecraft. The first challenge was to increase the light collection entrance aperture diameter, which was approximately 1 mm in the first prototype. The new design presented here increases this entrance aperture diameter to 4.2 mm, which is equivalent to a more than 16 times larger collection area. One of the trades made in realizing this improvement was to restrict the field-of-view to +80 deg. elevation and 360 azimuth. This trade stems from practical considerations where laser beam propagation over the excessively high air mass, which is in the line of sight (LOS) at low elevation angles, results in vulnerability to severe atmospheric turbulence and attenuation. An additional benefit of the new design is that the large entrance aperture is maintained even at large off-axis angles when the optic is pointed at zenith. The second critical limitation for implementing spectral filtering in the design was tackled by collimating the light prior to focusing it onto the focal plane. This allows the placement of the narrow spectral filter in the collimated portion of the beam. For the narrow band spectral filter to function properly, it is necessary to adequately control the range of incident angles at which received light intercepts the filter. When this angle is restricted via collimation, narrower spectral filtering can be implemented. The collimated beam (and the filter) must be relatively large to

  19. Chromospheric extents predicted by time-dependent acoustic wave models

    NASA Astrophysics Data System (ADS)

    Cuntz, Manfred

    1990-01-01

    Theoretical models for chromospheric structures of late-type giant stars are computed, including the time-dependent propagation of acoustic waves. Models with short-period monochromatic shock waves as well as a spectrum of acoustic waves are discussed, and the method is applied to the stars Arcturus, Aldebaran, and Betelgeuse. Chromospheric extent, defined as the monotonic decrease with height of the time-averaged electron densities, are found to be 1.12, 1.13, and 1.22 stellar radii for the three stars, respectively; this corresponds to a time-averaged electron density of 10 to the 7th/cu cm. Predictions of the extended chromospheric obtained using a simple scaling law agree well with those obtained by the time-dependent wave models; thus, the chromospheres of all stars for which the scaling law is valid consist of the same number of pressure scale heights.

  20. Chromospheric extents predicted by time-dependent acoustic wave models

    SciTech Connect

    Cuntz, M. Heidelberg Universitaet )

    1990-01-01

    Theoretical models for chromospheric structures of late-type giant stars are computed, including the time-dependent propagation of acoustic waves. Models with short-period monochromatic shock waves as well as a spectrum of acoustic waves are discussed, and the method is applied to the stars Arcturus, Aldebaran, and Betelgeuse. Chromospheric extent, defined as the monotonic decrease with height of the time-averaged electron densities, are found to be 1.12, 1.13, and 1.22 stellar radii for the three stars, respectively; this corresponds to a time-averaged electron density of 10 to the 7th/cu cm. Predictions of the extended chromospheric obtained using a simple scaling law agree well with those obtained by the time-dependent wave models; thus, the chromospheres of all stars for which the scaling law is valid consist of the same number of pressure scale heights. 74 refs.

  1. Time dependent flare model with non-LTE radiative transfer

    NASA Astrophysics Data System (ADS)

    Varady, M.; Karlický, M.; Kašparová, J.; Heinzel, P.

    2002-12-01

    The first results of a time dependent simulation of chromospheric response to a high energy electron beam are presented. The hybrid code, i.e. a combination of a 1-D hydrodynamic code and a test particle code, has been used to calculate the energy losses of a high energy electron beam propagating through the solar atmosphere and the consequent response of the ambient solar plasma to the energy deposition. The resulting time evolution of the solar plasma temperature, density, velocity and energy deposit on hydrogen has then been used as an input for a time dependent radiative transfer code in the MALI approach to determine the time variation of the Hα line profile. Non-thermal collisional rates have been included in the linearised ESE.

  2. Time-dependent response of filamentary composite spherical pressure vessels

    NASA Technical Reports Server (NTRS)

    Dozier, J. D.

    1983-01-01

    A filamentary composite spherical pressure vessel is modeled as a pseudoisotropic (or transversely isotropic) composite shell, with the effects of the liner and fill tubes omitted. Equations of elasticity, macromechanical and micromechanical formulations, and laminate properties are derived for the application of an internally pressured spherical composite vessel. Viscoelastic properties for the composite matrix are used to characterize time-dependent behavior. Using the maximum strain theory of failure, burst pressure and critical strain equations are formulated, solved in the Laplace domain with an associated elastic solution, and inverted back into the time domain using the method of collocation. Viscoelastic properties of HBFR-55 resin are experimentally determined and a Kevlar/HBFR-55 system is evaluated with a FORTRAN program. The computed reduction in burst pressure with respect to time indicates that the analysis employed may be used to predict the time-dependent response of a filamentary composite spherical pressure vessel.

  3. Statistical time-dependent model for the interstellar gas

    NASA Technical Reports Server (NTRS)

    Gerola, H.; Kafatos, M.; Mccray, R.

    1974-01-01

    We present models for temperature and ionization structure of low, uniform-density (approximately 0.3 per cu cm) interstellar gas in a galactic disk which is exposed to soft X rays from supernova outbursts occurring randomly in space and time. The structure was calculated by computing the time record of temperature and ionization at a given point by Monte Carlo simulation. The calculation yields probability distribution functions for ionized fraction, temperature, and their various observable moments. These time-dependent models predict a bimodal temperature distribution of the gas that agrees with various observations. Cold regions in the low-density gas may have the appearance of clouds in 21-cm absorption. The time-dependent model, in contrast to the steady-state model, predicts large fluctuations in ionization rate and the existence of cold (approximately 30 K), ionized (ionized fraction equal to about 0.1) regions.

  4. Transcriptional dynamics with time-dependent reaction rates

    NASA Astrophysics Data System (ADS)

    Nandi, Shubhendu; Ghosh, Anandamohan

    2015-02-01

    Transcription is the first step in the process of gene regulation that controls cell response to varying environmental conditions. Transcription is a stochastic process, involving synthesis and degradation of mRNAs, that can be modeled as a birth-death process. We consider a generic stochastic model, where the fluctuating environment is encoded in the time-dependent reaction rates. We obtain an exact analytical expression for the mRNA probability distribution and are able to analyze the response for arbitrary time-dependent protocols. Our analytical results and stochastic simulations confirm that the transcriptional machinery primarily act as a low-pass filter. We also show that depending on the system parameters, the mRNA levels in a cell population can show synchronous/asynchronous fluctuations and can deviate from Poisson statistics.

  5. Time-dependent buoyant puff model for explosive sources

    SciTech Connect

    Kansa, E.J.

    1997-01-01

    Several models exist to predict the time dependent behavior of bouyant puffs that result from explosions. This paper presents a new model that is derived from the strong conservative form of the conservation partial differential equations that are integrated over space to yield a coupled system of time dependent nonlinear ordinary differential equations. This model permits the cloud to evolve from an intial spherical shape not an ellipsoidal shape. It ignores the Boussinesq approximation, and treats the turbulence that is generated by the puff itself and the ambient atmospheric tubulence as separate mechanisms in determining the puff history. The puff cloud rise history was found to depend no only on the mass and initial temperature of the explosion, but also upon the stability conditions of the ambient atmosphere. This model was calibrated by comparison with the Roller Coaster experiments.

  6. Boosting thermoelectric efficiency using time-dependent control

    PubMed Central

    Zhou, Hangbo; Thingna, Juzar; Hänggi, Peter; Wang, Jian-Sheng; Li, Baowen

    2015-01-01

    Thermoelectric efficiency is defined as the ratio of power delivered to the load of a device to the rate of heat flow from the source. Till date, it has been studied in presence of thermodynamic constraints set by the Onsager reciprocal relation and the second law of thermodynamics that severely bottleneck the thermoelectric efficiency. In this study, we propose a pathway to bypass these constraints using a time-dependent control and present a theoretical framework to study dynamic thermoelectric transport in the far from equilibrium regime. The presence of a control yields the sought after substantial efficiency enhancement and importantly a significant amount of power supplied by the control is utilised to convert the wasted-heat energy into useful-electric energy. Our findings are robust against nonlinear interactions and suggest that external time-dependent forcing, which can be incorporated with existing devices, provides a beneficial scheme to boost thermoelectric efficiency. PMID:26464021

  7. Sublinear scaling for time-dependent stochastic density functional theory

    SciTech Connect

    Gao, Yi; Neuhauser, Daniel; Baer, Roi; Rabani, Eran

    2015-01-21

    A stochastic approach to time-dependent density functional theory is developed for computing the absorption cross section and the random phase approximation (RPA) correlation energy. The core idea of the approach involves time-propagation of a small set of stochastic orbitals which are first projected on the occupied space and then propagated in time according to the time-dependent Kohn-Sham equations. The evolving electron density is exactly represented when the number of random orbitals is infinite, but even a small number (≈16) of such orbitals is enough to obtain meaningful results for absorption spectrum and the RPA correlation energy per electron. We implement the approach for silicon nanocrystals using real-space grids and find that the overall scaling of the algorithm is sublinear with computational time and memory.

  8. Coherent states and their time dependence in fractional dimensions

    NASA Astrophysics Data System (ADS)

    Thilagam, A.; Lohe, M. A.

    2007-08-01

    We construct representations of the Lie algebra \\mathfrak{su}(1,1) using representations of the momentum and position operators satisfying the R-deformed Heisenberg relations, in which the fractional dimension d and angular momentum ell appear as parameters. The Bargmann index κ, which characterizes representations of the positive discrete series of \\mathfrak{su}(1,1) , can take any positive value. We construct coherent states in fractional dimensions, in particular we extend the two well-known analytic representations of coherent states for \\mathfrak{su}(1,1) , Perelomov and Barut-Girardello states, from dimension one to any dimension d. We generalize this construction to time-dependent coherent states by means of the \\mathfrak{su}(1,1) symmetries of the quantum time-dependent harmonic oscillator in fractional dimensions. We investigate the uncertainty relations of the momentum and position operators with respect to these coherent states, and their dependence on the dimension.

  9. Generalization of DT equations for time dependent sources.

    PubMed

    Neri, Lorenzo; Tudisco, Salvatore; Musumeci, Francesco; Scordino, Agata; Fallica, Giorgio; Mazzillo, Massimo; Zimbone, Massimo

    2010-01-01

    New equations for paralyzable, non paralyzable and hybrid DT models, valid for any time dependent sources are presented. We show how such new equations include the equations already used for constant rate sources, and how it's is possible to correct DT losses in the case of time dependent sources. Montecarlo simulations were performed to compare the equations behavior with the three DT models. Excellent accordance between equations predictions and Montecarlo simulation was found. We also obtain good results in the experimental validation of the new hybrid DT equation. Passive quenched SPAD device was chosen as a device affected by hybrid DT losses and active quenched SPAD with 50 ns DT was used as DT losses free device.

  10. The Role of Environment on Time Dependent Crack Growth

    DTIC Science & Technology

    1981-12-01

    reaction control and transport control terms. More recently, Wei and Shim (41) have extended these terms to represent frequency and temperature effects in...accelerate time dependent crack growth under either static loading (SCC or HE) or dynamic loading conditions. In some cases, the rate controlling ...processes of these phenomena have been related to surface controlled reactions, while in other cases bulk reactions such as diffusion appear to be rate

  11. Autoionization in time-dependent density-functional theory

    NASA Astrophysics Data System (ADS)

    Kapoor, V.

    2016-06-01

    We compute the exact exchange-correlation potential of the time-dependent density-functional theory (TDDFT) for the correlated process of autoionization. The potential develops barriers which regulate the autoionization rate. TDDFT employing known and practicable exchange-correlation potentials does not capture any autoionization dynamics. Approximate exchange-correlation potentials capturing such dynamics would necessarily require memory effects and are unlikely to be developed, as will be illustrated.

  12. Excitons in Time-Dependent Density-Functional Theory.

    PubMed

    Ullrich, Carsten A; Yang, Zeng-hui

    2016-01-01

    This chapter gives an overview of the description of the optical and dielectric properties of bulk insulators and semiconductors in time-dependent density-functional theory (TDDFT), with an emphasis on excitons. We review the linear-response formalism for periodic solids, discuss excitonic exchange-correlation kernels, calculate exciton binding energies for various materials, and compare the treatment of excitons with TDDFT and with the Bethe-Salpeter equation.

  13. Relating Time-Dependent Acceleration and Height Using an Elevator

    ERIC Educational Resources Information Center

    Kinser, Jason M.

    2015-01-01

    A simple experiment in relating a time-dependent linear acceleration function to height is explored through the use of a smartphone and an elevator. Given acceleration as a function of time, a(t), the velocity function and position functions are determined through integration as in v(t)=? a(t) dt (1) and x(t)=? v(t) dt. Mobile devices such as…

  14. Spectral methods for time dependent partial differential equations

    NASA Technical Reports Server (NTRS)

    Gottlieb, D.; Turkel, E.

    1983-01-01

    The theory of spectral methods for time dependent partial differential equations is reviewed. When the domain is periodic Fourier methods are presented while for nonperiodic problems both Chebyshev and Legendre methods are discussed. The theory is presented for both hyperbolic and parabolic systems using both Galerkin and collocation procedures. While most of the review considers problems with constant coefficients the extension to nonlinear problems is also discussed. Some results for problems with shocks are presented.

  15. Time Dependent Models of Grain Formation Around Carbon Stars

    NASA Technical Reports Server (NTRS)

    Egan, M. P.; Shipman, R. F.

    1996-01-01

    Carbon-rich Asymptotic Giant Branch stars are sites of dust formation and undergo mass loss at rates ranging from 10(exp -7) to 10(exp -4) solar mass/yr. The state-of-the-art in modeling these processes is time-dependent models which simultaneously solve the grain formation and gas dynamics problem. We present results from such a model, which also includes an exact solution of the radiative transfer within the system.

  16. The time dependence of molecular iodine emission from Laminaria digitata

    NASA Astrophysics Data System (ADS)

    Dixneuf, S.; Ruth, A. A.; Vaughan, S.; Varma, R. M.; Orphal, J.

    2009-02-01

    We present the first in situ detection of molecular iodine emitted from the brown macroalga Laminaria digitata under natural stress conditions. We show that the release of I2 occurs in short, strong bursts with a complex time signature. The new data indicate that algal control of I2 release in the form of an oscillatory time-dependence may be based on a nonlinear autocatalytic reaction scheme which is closely linked to the production of H2O2.

  17. The time dependence of molecular iodine emission from Laminaria digitata

    NASA Astrophysics Data System (ADS)

    Dixneuf, S.; Ruth, A. A.; Vaughan, S.; Varma, R. M.; Orphal, J.

    2008-08-01

    We present the first in situ detection of molecular iodine emitted from the brown macroalga Laminaria digitata under natural stress conditions. We show that the release of I2 occurs in short, strong bursts with a complex time signature. The new data indicate that algal control of I2 release in the form of an oscillatory time-dependence may be based on a nonlinear autocatalytic reaction scheme which is closely linked to the production of H2O2.

  18. Quantum anholonomies in time-dependent Aharonov-Bohm rings

    SciTech Connect

    Tanaka, Atushi; Cheon, Taksu

    2010-08-15

    Anholonomies in eigenstates are studied through time-dependent variations of a magnetic flux in an Aharonov-Bohm ring. The anholonomies in the eigenenergy and the expectation values of eigenstates are shown to persist beyond the adiabatic regime. The choice of the gauge of the magnetic flux is shown to be crucial to clarify the relationship of these anholonomies to the eigenspace anholonomy, which is described by a non-Abelian connection in the adiabatic limit.

  19. Brans-Dicke cosmology with time-dependent cosmological term

    NASA Astrophysics Data System (ADS)

    Berman, Marcelo Samuel

    1990-12-01

    Berman and Som's solution for a Brans-Dicke cosmology with time-dependent cosmological term, Robertson-Walker metric, perfect fluid, and perfect gas law of state solves the horizon, homogeneity, and isotropy problems without requiring any unnatural fine tuning in the very early universe, thus being an alternative model to inflation. The model also does not need recourse to quantum cosmology, and solves the flatness and magnetic monopole problems.

  20. Time-Dependent Effect of Chlorhexidine Surgical Prep

    DTIC Science & Technology

    2011-10-15

    Time-dependent effect of chlorhexidine surgical prep D.J. Stinner*, C.A. Krueger, B.D. Masini, J.C. Wenke United States Army Institute of Surgical ...2011 by J.A. Child Available online 15 October 2011 Keywords: Chlorhexidine Surgical site infection s u m m a r y Despite continued advances in...preoperative preventive measures and aseptic technique, surgical site infections remain a problem. The purpose of this study was to evaluate the time