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Sample records for magnetization reversal properties

  1. Shape-tuned dynamic properties of magnetic nanoelements during magnetization reversal

    NASA Astrophysics Data System (ADS)

    Zhang, Guang-fu; Li, Zhi-xiong; Wang, Xi-guang; Nie, Yao-zhuang; Guo, Guang-hua

    2015-07-01

    We study the dynamic properties of magnetic nanoelements with tapered ends by using micromagnetic simulations. It is found that the spin-wave modes can be effectively manipulated by the element shape. With the increase of the end sharpness (described by tapering parameter h), the frequency of the spin-wave edge mode increases rapidly and its oscillation areas in the both ends of element gradually increase and move toward to the central area. Finally, the edge mode completely merges into the fundamental mode. During the magnetization reversal processes, the edge mode experiences one or two softening depending on h≤60 nm or 60 nm100 nm, it is the fundamental mode that goes to zero at the switching field. The evolution of the spin-wave modes reflects the change of the micromagnetic structures of the elements during the reversal. It is the softening of the edge mode that triggers the magnetization reversal in elements with h<100 nm. The quasi-uniform reversal in the elements with h>100 nm is induced by the softening of the fundamental mode, where the edge mode is completely suppressed. The results presented in this work demonstrate that the dynamic properties and the magnetization reversal can be effectively tuned by changing the shape of the nanoelements and may be useful for designing the nanoscale magnetic devices.

  2. Magnetic properties of iron-based soft magnetic composites with SiO2 coating obtained by reverse microemulsion method

    NASA Astrophysics Data System (ADS)

    Wu, Shen; Sun, Aizhi; Lu, Zhenwen; Cheng, Chuan; Gao, Xuexu

    2015-05-01

    In this work, iron-based soft magnetic composites coated with the amorphous SiO2 layer have been fabricated by utilizing tetraethoxysilane in the reverse microemulsion method, and then the effects of addition amount of SiO2 and annealing temperature on the magnetic properties were investigated. The results show that the surface of iron powders contains a thin amorphous SiO2 insulation layer, which effectively decreases the magnetic loss of synthesized magnets. The magnetic loss of coated samples decreased by 87.8% as compared with that of uncoated samples at 150 kHz. Magnetic measurements show that the sample with 1.25 wt% SiO2 has an acceptable real part and minimum imaginary part of permeability in comparison with other samples. Also, the annealing treatment increased the initial permeability, the maximum permeability and the magnetic induction and decreased the coercivity with increasing temperature in the range 300-600 °C. The results of the loss separation imply that the annealed SMCs have a higher hysteresis loss coefficient (k2) and lower eddy current loss coefficient (k3) as compared with the pure iron compacts after the same heat treatment due to the preservation of the SiO2 layer.

  3. Nanosecond magnetization reversal in nanocrystalline magnetic films

    NASA Astrophysics Data System (ADS)

    Rahman, I. Z.; Gandhi, A. A.; Khaddem-Mousavi, M. V.; Lynch, T. F.; Rahman, M. A.

    2007-03-01

    This paper reports on the investigation of dynamic magnetization reversal process in electrodeposited nanocrystalline Ni and Ni80Fe20 films by employing nanosecond magnetic pulse technique. The surface morphology has been investigated using SEM, EDAX, XRD and AFM analyses and static magnetic properties of the films are characterized by vibrating sample magnetometer (VSM). Two different techniques are designed and employed to study the nanosecond magnetization reversal process in nanocrystalline thin films: Magneto-Optical Kerr Effect (MOKE) and nanosecond pulsed field magnetometer. Results of dynamical behavior as a function of several variables such as magnitude of applied bias magnetic field, amplitude and width of the pulsed magnetic field are analyzed in detail using both techniques. A computer simulation package called Object Oriented Micro-Magnetic Framework (OOMMF) has been used to simulate the magnetic domain patterns of the samples.

  4. Magnetic properties of pulse-reverse electrodeposited nanocrystalline NiFe/Cu composite wires in relation to the anodic current

    NASA Astrophysics Data System (ADS)

    Seet, H. L.; Li, X. P.; Lee, K. S.; Chia, H. Y.; Zheng, H. M.; Ng, W. C.

    2007-12-01

    Ni80Fe20/Cu composite wires were developed using the pulse-reverse electrodeposition technique with the cathodic (positive) current Ic fixed at 1 mA and the anodic (negative) current IA varied from 10 to 90% of Ic. The relationship between the magnetic properties of pulse reverse electrodeposited nanocrystalline NiFe/Cu composite wires and the anodic current was investigated. The results showed that the smaller the magnitude of the anodic current, the smaller was the average nanocrystalline grain size of the deposited material and the better was the uniformity of the surface, and consequently, the better the magnetic properties.

  5. Reversible collisionless magnetic reconnection

    SciTech Connect

    Ishizawa, A.; Watanabe, T.-H.

    2013-10-15

    Reversible magnetic reconnection is demonstrated for the first time by means of gyrokinetic numerical simulations of a collisionless magnetized plasma. Growth of a current-driven instability in a sheared magnetic field is accompanied by magnetic reconnection due to electron inertia effects. Following the instability growth, the collisionless reconnection is accelerated with development of a cross-shaped structure of current density, and then all field lines are reconnected. The fully reconnected state is followed by the secondary reconnection resulting in a weakly turbulent state. A time-reversed simulation starting from the turbulent state manifests that the collisionless reconnection process proceeds inversely leading to the initial state. During the reversed reconnection, the kinetic energy is reconverted into the original magnetic field energy. In order to understand the stability of reversed process, an external perturbation is added to the fully reconnected state, and it is found that the accelerated reconnection is reversible when the deviation of the E × B streamlines due to the perturbation is comparable with or smaller than a current layer width.

  6. Characterizing the Magnetic Properties of Natural Samples Using First-Order Reversal Curve Diagrams

    NASA Astrophysics Data System (ADS)

    Pike, C. R.; Roberts, A. P.; Verosub, K. L.

    2001-12-01

    A FORC diagram is calculated from a class of partial hysteresis curves known as first-order reversal curves or FORCs. The measurement of a FORC begins by saturating a sample in a large positive applied field. The field is then decreased to a specified field and reversed; the FORC consists of the magnetization curve that results when the applied field is increased from this reversal field back to saturation. By repeating this measurement for different reversal fields, one obtains a suite of curves that provide detailed information on the distribution of particle switching fields (coercivities) and interaction fields in the sample. These magnetization data are transformed into a FORC distribution by calculating a second derivative of the magnetization data, and by applying a change in co-ordinates. The FORC distribution is, therefore, an empirically well-defined quantity that can be used to probe subtle variations in hysteresis behavior. We have used FORC diagrams to characterize the main types of hysteresis behavior observed in rock magnetism and environmental magnetism. FORC diagrams can be calculated using room-temperature or low-temperature data and enable identification of superparamagnetic, single domain and multi-domain grains, as well as magnetostatic interactions, even in mixed magnetic mineral assemblages. Routine use of FORC diagrams to examine representative bulk samples from large sample collections can provide important information concerning the magnetic particles that cannot be obtained using standard hysteresis measurements. In addition to using FORC diagrams to identify specific magnetic components in a sample, they can also be used to understand fundamental problems in rock magnetism. Our results suggest that pseudo-single domain grains contain contributions from single domain and multi-domain moments and that the hysteresis behavior observed in the multi-domain grains typically encountered in rock magnetism cannot be solely explained through

  7. Effects of strain-induced martensite and its reversion on the magnetic properties of AISI 201 austenitic stainless steel

    NASA Astrophysics Data System (ADS)

    Souza Filho, I. R.; Sandim, M. J. R.; Cohen, R.; Nagamine, L. C. C. M.; Hoffmann, J.; Bolmaro, R. E.; Sandim, H. R. Z.

    2016-12-01

    Strain-induced martensite (SIM) and its reversion in a cold-rolled AISI 201 austenitic stainless steel was studied by means of magnetic properties, light optical (LOM) and scanning electron (SEM) microscopy, electron backscatter diffraction (EBSD), texture measurements, and Vickers microhardness testing. According to Thermo-calc© predictions, the BCC phase (residual δ-ferrite and SIM) is expected to be stable until 600 °C. The current material was cold rolled up to 60% thickness reduction and submitted to both isothermal and stepwise annealing up to 800 °C. Magnetic measurements were taken during annealing (in situ) of the samples and also for their post mortem conditions. The Curie temperatures (Tc) of residual δ-ferrite and SIM have similar values between 550 and 600 °C. Besides Tc, the focused magnetic parameters were saturation magnetization (Ms), remanent magnetization (MR), and coercive field (Hc). SIM reversion was found to occur in the range of 600-700 °C in good agreement with Thermo-calc© predictions. The microstructures of the material, annealed at 600 and 700 °C for 1 h, were investigated via EBSD. Microtexture measurements for these samples revealed that the texture components were mainly those found for the 60% cold rolled material. This is an evidence that the SIM reversion occurred by an athermal mechanism.

  8. Periodicity of the earth's magnetic reversals

    NASA Technical Reports Server (NTRS)

    Stothers, R. B.

    1986-01-01

    Results are presented from an attempt to perform a relatively comprehensive analysis of the evidence for a periodicity, with harmonics, of the observed regular reversals of the earth's magnetic field. The database considered covers 296 reversals over the past 165 Myr. Histograms with bins 1 Myr apart reveal only 30 Myr reversal patterns. The reversal dates are fitted to a linear periodic function and a spectrum is computed for the residuals at the adopted dates. The possible presence of multiple periodicities is evaluated and over various time intervals. The analysis shows that a recently observed 15 Myr periodicity is probably a harmonic of the 29.5-30.5 Myr period. The calculations do not confirm an inherent magnetic reversal property of the earth. The reversals may arise from tectonic events or from impacts from extraterrestrial objects.

  9. Ancient Magnetic Reversals: Clues to the Geodynamo.

    ERIC Educational Resources Information Center

    Hoffman, Kenneth A.

    1988-01-01

    Discusses the question posed by some that the earth's magnetic field may reverse. States that rocks magnetized by ancient fields may offer clues to the underlying reversal mechanism in the earth's core. (TW)

  10. Chemical and magnetic properties of rapidly cooled metastable ferri-ilmenite solid solutions - IV: the fine structure of self-reversed thermoremanent magnetization

    NASA Astrophysics Data System (ADS)

    Robinson, Peter; McEnroe, S. A.; Fabian, K.; Harrison, R. J.; Thomas, C. I.; Mukai, H.

    2014-03-01

    Magnetic experiments, a Monte Carlo simulation and transmission electron microscopy observations combine to confirm variable chemical phase separation during quench and annealing of metastable ferri-ilmenite compositions, caused by inhomogeneous Fe-Ti ordering and anti-ordering. Separation begins near interfaces between growing ordered and anti-ordered domains, the latter becoming progressively enriched in ilmenite component, moving the Ti-impoverished hematite component into Fe-enriched diffusion waves near the interfaces. Even when disordered regions are eliminated, Fe-enriched waves persist and enlarge on anti-phase boundaries between growing and shrinking ordered and anti-ordered domains. Magnetic results and conceptual models show that magnetic ordering with falling T initiates in the Fe-enriched wave crests. Although representing only a tiny fraction of material, identified at highest Ts on a field-cooling curve, they control the `pre-destiny' of progressive magnetization at lower T. They can provide a positive magnetic moment in a minority of ordered ferrimagnetic material, which, by exchange coupling, then creates a self-reversed negative moment in the remaining majority. Four Ts or T ranges are recognized on typical field-cooling curves: TPD is the T range of `pre-destination'; TC is the predominant Curie T where major positive magnetization increases sharply; TMAX is where magnetization reaches a positive maximum, beyond which it is outweighed by self-reversed magnetization and TZM is the T where total magnetization passes zero. Disposition of these Ts on cooling curves indicate the fine structure of self-reversed thermoremanent magnetization. These results confirm much earlier suspicions that the `x-phase' responsible for self-reversed magnetization resides in Fe-enriched phase boundaries.

  11. Magnetic properties of hemoilmenite single crystals in Haruna dacite pumice revealed by the Bitter technique, with special reference to self-reversal of thermoremanent magnetization

    NASA Astrophysics Data System (ADS)

    Ozima, M.; Funaki, M.

    2001-02-01

    In order to reconsider the mechanism of the self-reversal of TRM (SRTRM) of hemoilmenite in dacite pumice, magnetic properties of newly collected Haruna dacite pumice near the historical sampling site (more than 50 years ago) were investigated again. All Haruna dacite pumice samples collected showed SRTRM or at least partial SRTRM. This time, the methods of microprobe analysis and the Bitter technique which were not available 50 years ago, were added to examine hemoilmenite crystals. Contrary to the result which was first reported by Hoffmann and Fehr on the basis of the micromagnetic observation of hemoilmenite crystals in Pinatubo dacite pumice, our hemoilmenite crystals are considerably more homogeneous in TiO2-content in a single crystal than those of Hoffmann and Fehr. Also, we could not find any "shell structure" with two phases having different magnetism and compositions in a single crystal of hemoilmenite in Haruna dacite pumice. We came to the conclusion that the intergrown shell-structure itself in Hoffmann and Fehr's model may not be essential but only the coexistence of the intergrown two phases in a single crystal of hemoilmenite must be essential for the acquisition of SRTRM of hemoilmenite. Both models, one by Ishikawa and Syono and the other by Hoffmann and Fehr are basically similar to each other, regardless of the structure involved.

  12. Magnetization reversal in exchange biased nanocap arrays

    NASA Astrophysics Data System (ADS)

    Guhr, I. L.; van Dijken, S.; Malinowski, G.; Fischer, P.; Springer, F.; Hellwig, O.; Albrecht, M.

    2007-05-01

    Arrays of self-assembled polystyrene spheres with various particle sizes have been used as a substrate to study the exchange bias effect along the out-of-plane direction of Pt/Co multilayers capped with IrMn layers. The evolution of the reversal process of the resulting magnetic nanocaps was investigated by magnetic force microscopy (MFM) and magnetic transmission x-ray microscopy (M-TXM). Tip-sample interaction-induced irreversible and reversible switching events have been observed during multiple scanning cycles in MFM imaging which are ascribed to the so-called training effect. During M-TXM imaging a drastic change in morphology has been found due to the x-ray exposure, leading to the formation of much larger spherical particles. Interestingly, these merged particles reveal again an exchange coupled single-domain magnetic cap with magnetic behaviour similar to magnetic films deposited directly on spheres of similar size. This paper was presented at the Materials Research Society Fall 2006 Meeting, 27 November-1 December 2006, as part of Symposium P: Nanoscale Magnets-Synthesis, Self-assembly, Properties and Applications, organized by J Fassbender, J Chapman and C A Ross.

  13. Chemical and magnetic properties of rapidly cooled metastable ferri-ilmenite solid solutions: implications for magnetic self-reversal and exchange bias—I. Fe-Ti order transition in quenched synthetic ilmenite 61

    NASA Astrophysics Data System (ADS)

    Fabian, Karl; Miyajima, Nobuyoshi; Robinson, Peter; McEnroe, Suzanne A.; Ballaran, Tiziana Boffa; Burton, Benjamin P.

    2011-09-01

    Quenched ferri-ilmenite solid solutions X FeTiO3+ (1 -X) Fe2O3 with X≈ 0.60 contain chemical and magnetic structures important for understanding the unusual magnetic properties in this series, including self-reversal in igneous rocks and exchange bias. Here we study a composition X= 0.61, annealed at 1055 °C, above the Fe-Ti ordering temperature, then quenched. Presence of two interface-coupled phases is established by pot-bellied character of the room-temperature magnetic hysteresis loop, and large negative magnetic exchange bias below 30 K. Transmission electron microscopy (TEM) dark-field imaging with the 003 reflection shows dominant Fe-Ti disordered antiferromagnetic and lesser ordered ferrimagnetic phases, the latter in lenses ≤8 nm thick. Parts of the ordered phase are in antiphase relationship, shown by high-resolution TEM imaging of Fe-rich and Ti-rich layers. TEM-EDX analyses indicate chemical phase separation during quench, with dominant compositions X= 0.56-0.63, extremes 0.50 and 0.70. Thermomagnetic experiments indicate compositions X= 0.56-0.61 are antiferromagnetic, X= 0.61-0.64 are ferrimagnetic. A sample held ˜5 min at 1063 K, increased in order, demonstrated by twofold increase in induced moment at 1 T. This then acquired self-reversed thermoremanent magnetization between 490 and 440 K. Progressive annealings of another sample at 773 K, 973 K, 1023 K and 1063 K, followed by cooling in a 1 T field, produced positive room-temperature magnetic exchange bias, only for 1023 K and 1063 K runs. These properties suggest growth of ordered regions from disordered regions, and expansion of some ordered domains against others across antiphase boundaries, thus creating self-organized structures essential for magnetic self-reversal and magnetic exchange bias.

  14. Magnetization ground state and reversal modes of magnetic nanotori

    NASA Astrophysics Data System (ADS)

    Vojkovic, Smiljan; Nunez, Alvaro S.; Altbir, Dora; Carvalho-Santos, Vagson L.

    2016-07-01

    In this work, and by means of micromagnetic simulations, we study the magnetic properties of toroidal nanomagnets. The magnetization ground state for different values of the aspect ratio between the toroidal and polar radii of the nanotorus has been obtained. Besides, we have shown that the vortex and the in-plane single domain states can appear as ground states for different ranges of the aspect ratio, while a single domain state with an out-of-plane magnetization is not observed. The hysteresis curves are also obtained, evidencing the existence of two reversal modes depending on the geometry: a vortex mode and a coherent rotation. A comparison between toroidal and cylindrical nanoparticles has been performed evidencing that nanotori can accommodate a vortex as the ground state for smaller volume than cylindrical nanorings.

  15. Magnetization reversal properties of Pr{sub 1-x}(Gd/Nd){sub x}MnO{sub 3} (x=0.3, 0.5, 0.7)

    SciTech Connect

    Biswas, Sanjay; Pal, Sudipta; Bose, Esa

    2015-06-24

    We report measurements of the temperature dependent magnetic properties of single phase orthorhombic perovskites system associated with space group Pbnm compounds Pr{sub 1-x}(Gd/Nd){sub x}MnO{sub 3} (x=0.3, 0.5, 0.7). Magnetic properties radically changes with the doping of Gd or Nd. A magnetization reversal is observed below the Neel temperature (T{sub N}), in DC magnetization measurements (at 50 Oe) in the doped compounds. The reversal of magnetization may be due to the antiparallel coupling between the two magnetic sublattices (|Pr+ Gd/ Nd | and Mn). The hysteresis plot taken at 50K indicates a ferrimagnetic characteristic and existence of spin canting of ions in the magnetic sublattices.

  16. Magnetic vortex state stability, reversal and dynamics in restricted geometries.

    PubMed

    Guslienko, K Yu

    2008-06-01

    Magnetic vortices are typically the ground states in geometrically confined ferromagnets with small magnetocrystalline anisotropy. In this article I review static and dynamic properties of the magnetic vortex state in small particles with nanoscale thickness and sub-micron and micron lateral sizes (magnetic dots). Magnetic dots made of soft magnetic material shaped as flat circular and elliptic cylinders are considered. Such mesoscopic dots undergo magnetization reversal through successive nucleation, displacement and annihilation of magnetic vortices. The reversal process depends on the stability of different possible zero-field magnetization configurations with respect to the dot geometrical parameters and application of an external magnetic field. The interdot magnetostatic interaction plays an important role in magnetization reversal for dot arrays with a small dot-to-dot distance, leading to decreases in the vortex nucleation and annihilation fields. Magnetic vortices reveal rich, non-trivial dynamical properties due to existance of the vortex core bearing topological charges. The vortex ground state magnetization distribution leads to a considerable modification of the nature of spin excitations in comparison to those in the uniformly magnetized state. A magnetic vortex confined in a magnetically soft ferromagnet with micron-sized lateral dimensions possesses a characteristic dynamic excitation known as a translational mode that corresponds to spiral-like precession of the vortex core around its equilibrium position. The translation motions of coupled vortices are considered. There are, above the vortex translation mode eigenfrequencies, several dynamic magnetization eigenmodes localized outside the vortex core whose frequencies are determined principally by dynamic demagnetizing fields appearing due to restricted dot geometry. The vortex excitation modes are classified as translation modes and radially or azimuthally symmetric spin waves over the vortex

  17. Anomalous spontaneous reversal in magnetic heterostructures.

    PubMed

    Li, Zhi-Pan; Eisenmenger, Johannes; Miller, Casey W; Schuller, Ivan K

    2006-04-01

    We observe a thermally induced spontaneous magnetization reversal of epitaxial ferromagnet/antiferromagnet heterostructures under a constant applied magnetic field. Unlike any other magnetic system, the magnetization spontaneously reverses, aligning antiparallel to an applied field with decreasing temperature. We show that this unusual phenomenon is caused by the interfacial antiferromagnetic coupling overcoming the Zeeman energy of the ferromagnet. A significant temperature hysteresis exists, whose height and width can be tuned by the field applied during thermal cycling. The hysteresis originates from the intrinsic magnetic anisotropy in the system. The observation of this phenomenon leads to open questions in the general understanding of magnetic heterostructures. Moreover, this shows that in general heterogeneous nanostructured materials may exhibit unexpected phenomena absent in the bulk.

  18. Atomic structure and magnetic properties of MnFe2O4 nanoparticles produced by reverse micelle synthesis

    NASA Astrophysics Data System (ADS)

    Carpenter, Everett E.; O'Connor, Charles J.; Harris, Vincent G.

    1999-04-01

    Using the aqueous cores of reverse micelles as nanoreactors, nanoparticles (d˜10 nm) of the mixed ferrite MnFe2O4 were produced. Seven processing trials were performed where the concentration of ammonium hydroxide, reaction temperature, and the oxidizing agent were varied. All trials result in Mn-ferrite particles with varying chemistry and structure. The Mn concentration in the resulting ferrite is strongly enhanced by both the presence of H2O2 as an oxidizing agent and a surplus of ammonium hydroxide. The increased Mn concentration correlates with a higher fraction of octahedrally coordinated Mn cations. When near-stoic amounts of ammonium hydroxide are used, the resulting ferrites are nearly stoichiometric with a more equitable distribution of Mn cations on the octahedral and tetrahedral sublattices. In all ferrite nanoparticles, the Mn cations have a preference for octahedral site occupancy that is larger than the 20% measured in bulk Mn-ferrite. We attribute the cation filling trends to the stabilization of excess trivalent Mn during processing.

  19. Magnetization reversal driven by a spin torque oscillator

    SciTech Connect

    Sbiaa, R.

    2014-09-01

    Magnetization reversal of a magnetic free layer under spin transfer torque (STT) effect from a magnetic hard layer with a fixed magnetization direction and an oscillating layer is investigated. By including STT from the oscillating layer with in-plane anisotropy and orthogonal polarizer, magnetization-time dependence of free layer is determined. The results show that the frequency and amplitude of oscillations can be varied by adjusting the current density and magnetic properties. For an optimal oscillation frequency (f{sub opt}), a reduction of the switching time (t{sub 0}) of the free layer is observed. Both f{sub opt} and t{sub 0} increase with the anisotropy field of the free layer.

  20. Magnetic reversals in a modified shell model for magnetohydrodynamics turbulence

    NASA Astrophysics Data System (ADS)

    Nigro, Giuseppina; Carbone, Vincenzo

    2010-07-01

    The aim of the paper is the study of dynamo action using a simple nonlinear model in the framework of magnetohydrodynamic turbulence. The nonlinear behavior of the system is described by using a shell model for velocity field and magnetic field fluctuations, modified for the magnetic field at the largest scale by a term describing a supercritical pitchfork bifurcation. Turbulent fluctuations generate a dynamical situation where the large-scale magnetic field jumps between two states which represent the opposite polarities of the magnetic field. Despite its simplicity, the model has the capability to describe a long time series of reversals from which we infer results about the statistics of persistence times and scaling laws of cancellations between opposite polarities for different magnetic diffusivity coefficients. These properties of the model are compared with real paleomagnetic data, thus revealing the origin of long-range correlations in the process.

  1. Effect of high-frequency driving current on magnetization reversal in Co-rich amorphous microwires

    SciTech Connect

    Chizhik, A.; Zhukov, A.; Gonzalez, J.; Blanco, J.M.

    2004-09-20

    Influence of high frequency electric current on the magnetization reversal in Co-rich glass covered amorphous microwires has been studied. The strong correlation between the coercivity and the circular magnetization in the outer shell of the wire has been found. The change of the mechanism of magnetization reversal in the presence of high-frequency circular magnetic field, which is related with the impedance properties, is presented.

  2. TOPICAL REVIEW: Electrical magnetization reversal in ferromagnetic III V semiconductors

    NASA Astrophysics Data System (ADS)

    Chiba, D.; Matsukura, F.; Ohno, H.

    2006-07-01

    Introduction of a high concentration of manganese in III-V semiconductors, such as InAs and GaAs, results in carrier-induced ferromagnetism, which allows us to integrate ferromagnetism in nonmagnetic heterostructures and which modifies their magnetic properties through electric-field control of carrier concentration. The properties of ferromagnetism can in many cases be semi-quantitatively understood by the p-d Zener model, which is qualitatively different from conventional ferromagnetic metals. These ferromagnetic III-V semiconductors also offer the unique opportunity of examining spin-dependent phenomena observed so far only in metallic systems. Here, we review our experimental study on electrical manipulation of magnetization in these ferromagnetic III-V semiconductors. We first describe the results of electrically assisted magnetization reversal in ferromagnetic semiconductor (In, Mn)As field-effect transistor structures. The coercivity as well as ferromagnetic transition temperature can be controlled through the modification of carrier concentration by applied electric fields in a gated structure. We then present electrical magnetization reversal by spin-transfer torque exerted by spin-polarized currents at low threshold current density (~105 A cm-2) in (Ga, Mn)As-based magnetic tunnel junctions.

  3. Lightweight Magnetic Cooler With a Reversible Circulator

    NASA Technical Reports Server (NTRS)

    Chen, Weibo; McCormick, John

    2011-01-01

    A design of a highly efficient and lightweight space magnetic cooler has been developed that can continuously provide remote/distributed cooling at temperatures in the range of 2 K with a heat sink at about 15 K. The innovative design uses a cryogenic circulator that enables the cooler to operate at a high cycle frequency to achieve a large cooling capacity. The ability to provide remote/distributed cooling not only allows flexible integration with a payload and spacecraft, but also reduces the mass of the magnetic shields needed. The active magnetic regenerative refrigerator (AMRR) system is shown in the figure. This design mainly consists of two identical magnetic regenerators surrounded by their superconducting magnets and a reversible circulator. Each regenerator also has a heat exchanger at its warm end to reject the magnetization heat to the heat sink, and the two regenerators share a cold-end heat exchanger to absorb heat from a cooling target. The circulator controls the flow direction, which cycles in concert with the magnetic fields, to facilitate heat transfer. Helium enters the hot end of the demagnetized column, is cooled by the refrigerant, and passes into the cold-end heat exchanger to absorb heat. The helium then enters the cold end of the magnetized column, absorbing heat from the refrigerant, and enters the hot-end heat exchanger to reject the magnetization heat. The efficient heat transfer in the AMRR allows the system to operate at a relatively short cycle period to achieve a large cooling power. The key mechanical components in the magnetic cooler are the reversible circulator and the magnetic regenerators. The circulator uses non-contacting, self-acting gas bearings and clearance seals to achieve long life and vibration- free operation. There are no valves or mechanical wear in this circulator, so the reliability is predicted to be very high. The magnetic regenerator employs a structured bed configuration. The core consists of a stack of thin

  4. Magnetic properties of electrodeposited nanowires

    NASA Astrophysics Data System (ADS)

    Heydon, G. P.; Hoon, S. R.; Farley, A. N.; Tomlinson, S. L.; Valera, M. S.; Attenborough, K.; Schwarzacher, W.

    1997-04-01

    Electrodeposited multilayered nanowires grown within a polycarbonate membrane constitute a new medium in which giant magnetoresistance (GMR) perpendicular to the plane of the multilayers can be measured. These structures can exhibit a perpendicular GMR of at least 22% at ambient temperature. We performed detailed studies both of reversible magnetization and of irreversible remanent magnetization curves for CoNiCu/Cu/CoNiCu multilayered and CoNiCu pulse-deposited nanowire systems with Co:Ni ratios of 6:4 and 7:3 respectively in the range 10 - 290 K, allowing the magnetic phases of these structures to be identified. Shape anisotropy in the pulse-deposited nanowire and inter-layer coupling in the multilayered nanowire are shown to make important contributions to the magnetic properties. Dipolar-like interactions are found to predominate in both nanowire systems. Magnetic force microscope (MFM) images of individual multilayered nanowires exhibit a contrast consistent with there being a soft magnetization parallel to the layers. Switching of the magnetic layers in the multilayered structure into the direction of the MFM tip's stray field is observed.

  5. Control of magnetization reversal in oriented strontium ferrite thin films

    SciTech Connect

    Roy, Debangsu Anil Kumar, P. S.

    2014-02-21

    Oriented Strontium Ferrite films with the c axis orientation were deposited with varying oxygen partial pressure on Al{sub 2}O{sub 3}(0001) substrate using Pulsed Laser Deposition technique. The angle dependent magnetic hysteresis, remanent coercivity, and temperature dependent coercivity had been employed to understand the magnetization reversal of these films. It was found that the Strontium Ferrite thin film grown at lower (higher) oxygen partial pressure shows Stoner-Wohlfarth type (Kondorsky like) reversal. The relative importance of pinning and nucleation processes during magnetization reversal is used to explain the type of the magnetization reversal with different oxygen partial pressure during growth.

  6. Magnetic field diffusion and dissipation in reversed-field plasmas

    NASA Technical Reports Server (NTRS)

    Drake, J. F.; Gladd, N. T.; Huba, J. D.

    1981-01-01

    A diffusion equation is derived which describes the evolution of a magnetic field in a plasma of arbitrary beta and resistivity. The equation is valid for a one-dimensional slab geometry, assumes the plasma remains in quasi-equilibrium throughout its evolution and does not include thermal transport. Scaling laws governing the rate of change of the magnetic energy, particle drift energy, and magnetic flux are calculated. It is found that the magnetic free energy can be substantially larger than the particle drift energy and can be an important energy reservoir in driving plasma instabilities (e.g., the lower-hybrid-drift instability). In addition, the effect of a spatially varying resistivity on the evolution of a reversed-field plasma is studied. The resistivity model used is based upon the anomalous transport properties associated with the nonlocal mode structure of the lower-hybrid-drift instability. The relevance of this research to laboratory plasmas (e.g., theta pinches, reversed-field theta pinches) and space plasmas (e.g., the earth's magnetotail) is discussed.

  7. Chondrule magnetic properties

    NASA Technical Reports Server (NTRS)

    Wasilewski, P. J.; Obryan, M. V.

    1994-01-01

    The topics discussed include the following: chondrule magnetic properties; chondrules from the same meteorite; and REM values (the ratio for remanence initially measured to saturation remanence in 1 Tesla field). The preliminary field estimates for chondrules magnetizing environments range from minimal to a least several mT. These estimates are based on REM values and the characteristics of the remanence initially measured (natural remanence) thermal demagnetization compared to the saturation remanence in 1 Tesla field demagnetization.

  8. Magnetically actuated patterns for bioinspired reversible adhesion (dry and wet).

    PubMed

    Drotlef, Dirk-Michael; Blümler, Peter; del Campo, Aránzazu

    2014-02-01

    A facile strategy to obtain magnetically actuated arrays of micropillars able to undergo reversible, homogeneous, drastic, and tunable geometrical changes upon application of a magnetic field with variable strength is demonstrated. A magnetically tunable gecko-inspired adhesive that works under dry and wet conditions is realized using elastomeric micropatterns containing magnetic microparticles.

  9. Magnetic properties and vapochromic reversible guest-induced transformation in a bispyrazolato copper(II) polymer: an experimental and dispersion-corrected density functional theory study.

    PubMed

    Bencini, Alessandro; Casarin, Maurizio; Forrer, Daniel; Franco, Lorenzo; Garau, Federica; Masciocchi, Norberto; Pandolfo, Luciano; Pettinari, Claudio; Ruzzi, Marco; Vittadini, Andrea

    2009-05-01

    Dispersion-corrected density functional theory (DFT-D) calculations, Electron Spin Resonance spectroscopy (EPR), and variable temperature magnetic moment measurements were used to investigate the structure and the electronic/magnetic properties of bispyrazolato-copper(II) coordination polymer and of its hydration product. The Cu(II) ions are antiferromagnetically coupled through the sigma system of the pyrazolate rings in both compounds. Theoretical electron density maps reveal that water molecules interact simultaneously and to a comparable extent with two Cu(II) centers (through the electronegative O end) and two pyrazolate rings (through the partly positively charged H atoms), which is compatible with the observed internuclear distances. DFT-D calculations indicate that low kinetic barriers are involved in the rearrangement of the host structure.

  10. Ultralow field magnetization reversal of two-body magnetic nanoparticles

    NASA Astrophysics Data System (ADS)

    Li, Fei; Lu, Jincheng; Lu, Xiaofeng; Tang, Rujun; Sun, Z. Z.

    2016-08-01

    Field induced magnetization reversal was investigated in a system of two magnetic nanoparticles with uniaxial anisotropies and magnetostatic interaction. By using the micromagnetic simulation, ultralow switching field strength was found when the separation distance between the two particles reaches a critical small value (on nanometer scale) in the perpendicular configuration where the anisotropic axes of the two particles are perpendicular to the separation line. The switching field increases sharply when the separation is away from the critical distance. The ultralow field switching phenomenon was missed in the parallel configuration where both the anisotropic axes are aligned along the separation line of the two particles. The micromagnetic results are consistent with the previous theoretical prediction [J. Appl. Phys. 109, 104303 (2011)] where dipolar interaction between two single-domain magnetic particles was considered. Our present simulations offered further proofs and possibilities for the low-power applications of information storage as the two-body magnetic nanoparticles might be implemented as a composite information bit.

  11. Magnetically Responsive Nanostructures with Tunable Optical Properties.

    PubMed

    Wang, Mingsheng; Yin, Yadong

    2016-05-25

    Stimuli-responsive materials can sense specific environmental changes and adjust their physical properties in a predictable manner, making them highly desired components for designing novel sensors, intelligent systems, and adaptive structures. Magnetically responsive structures have unique advantages in applications, as external magnetic stimuli can be applied in a contactless manner and cause rapid and reversible responses. In this Perspective, we discuss our recent progress in the design and fabrication of nanostructured materials with various optical responses to externally applied magnetic fields. We demonstrate tuning of the optical properties by taking advantage of the magnetic fields' abilities to induce magnetic dipole-dipole interactions or control the orientation of the colloidal magnetic nanostructures. The design strategies are expected to be extendable to the fabrication of novel responsive materials with new optical effects and many other physical properties. PMID:27115174

  12. Micromagnetic calculation of magnetization reversal in magnetic rings

    NASA Astrophysics Data System (ADS)

    Lopez-Diaz, Luis

    2002-03-01

    The success of using patterned magnetic nanoelements in Magnetic Random Access Memories (MRAM) depends entirely on our ability to control accurately their switching fields. In a recent study1, we showed that micron-sized narrow rings present well defined stable states and nucleation-free switching between them. In the first part of the talk we review our experimental studies on ring magnets. Pre-patterned Si(100) substrates were used to grow free-standing epitaxial ring magnets of Cu(100)/Co(100)/Cu(100)/Si(100) with 1.8 mm outer diameter, 1.2 mm inner diameter and 34 nm thickness. The samples were magnetically characterised using specially adapted magneto-optic Kerr effect. The measurements show that a two step switching process occurs at high fields, indicating the existence of two different stable states. In addition to the vortex state, which occurs at intermediate fields, we have identified a second state which is also stable at remanence and undergoes a simple and well characterised nucleation free domain wall propagation switching process. Moreover, it is confirmed that the rings reverse by falling into vortex states with different circulation when the field is applied in opposite directions. This means a particular vortex state (clockwise or counter-clockwise) can be prepared using a uniform field only, which can be important for technological applications. In the second part of the talk we use micromagnetic simulations to further explore the potential performance of narrow rings as memory cells in MRAM devices in terms of scalability and switching speed. We introduce two artificial notches at the outer surface of the rings in order to control accurately the depinning fields for the domain walls. According to our simulations, well defined onion states1 and switching by domain wall motion can be achieved for ring diameters down 180 nm. In order to speed up the switching process, two different approaches are considered. In the first one, a field pulse is

  13. Magnetization reversal in TmCrO{sub 3}

    SciTech Connect

    Yoshii, Kenji

    2012-11-15

    Highlights: ► We observed two magnetization reversals in TmCrO{sub 3}. ► The reversal at 28 K is attributed to antiparallel coupling between Cr{sup 3+} and Tm{sup 3+}. ► The other reversal originates from spin reorientation. ► Magnetocaloric effect is observed at the spin reorientation temperature. ► Characteristic magnetization switching is demonstrated. -- Abstract: The perovskite chromite TmCrO{sub 3} shows magnetization reversal at two temperatures. The reversal at ∼28 K is attributed to the antiparallel coupling between Tm{sup 3+} and Cr{sup 3+} moments, while that at the lower temperature (∼6–7 K) is rooted in a rotation of the magnetic moments. Magnetocaloric measurements offer a relatively large entropy change (∼4–5 J kg{sup −1} K{sup −1}) at the lower temperature. The reversal at ∼28 K is accompanied by a sign change of an exchange-bias-like field. The absence of the training effect suggests that this behavior is rooted in unidirectional magnetic anisotropy. The existence of the two magnetization reversals offers the characteristic switching of magnetization. For example, the magnetization is flipped without changing the direction of the applied magnetic field.

  14. Full 180° Magnetization Reversal with Electric Fields

    PubMed Central

    Wang, J. J.; Hu, J. M.; Ma, J.; Zhang, J. X.; Chen, L. Q.; Nan, C. W.

    2014-01-01

    Achieving 180° magnetization reversal with an electric field rather than a current or magnetic field is a fundamental challenge and represents a technological breakthrough towards new memory cell designs. Here we propose a mesoscale morphological engineering approach to accomplishing full 180° magnetization reversals with electric fields by utilizing both the in-plane piezostrains and magnetic shape anisotropy of a multiferroic heterostructure. Using phase-field simulations, we examined a patterned single-domain nanomagnet with four-fold magnetic axis on a ferroelectric layer with electric-field-induced uniaxial strains. We demonstrated that the uniaxial piezostrains, if non-collinear to the magnetic easy axis of the nanomagnet at certain angles, induce two successive, deterministic 90° magnetization rotations, thereby leading to full 180° magnetization reversals. PMID:25512070

  15. Tailoring the magnetization reversal of elliptical dots using exchange bias.

    SciTech Connect

    Sort, J.; Buchanan, K. S.; Pearson, J. E.; Hoffmann, A.; Menendez, E.; Salazar-Alvarez, G.; Baro, M. D.; Miron, M.; Rodamcq, B.; Dieny, B.; ICREA; Univ. Autonoma of Barcelona; Insti. Catala de Nanotecnologia; SPINTEC

    2008-01-01

    Exchange bias effects have been studied in elliptical dots composed of ferromagnetic Ni{sub 80}Fe{sub 20}-antiferromagnetic Ir{sub 20}Mn{sub 80} bilayers. The magnetization reversal mechanisms and magnetic configurations have been investigated by magneto-optic Kerr effect and magnetic force microscopy. Although the obtained bias fields in these dots are relatively small, the magnetization reversal is found to be influenced by the ferromagnetic-antiferromagnetic coupling. Namely, for some off-axis angles of measurement, the magnetization reversal mechanism of the Ni{sub 80}Fe{sub 20}-Ir{sub 20}Mn{sub 80} ellipses depends on whether exchange bias is induced along the minor or major axis of the ellipses. Hence, exchange bias is shown to be an effective means for tailoring the magnetization reversal of elliptical dots after sample fabrication.

  16. Reversible aggregation and magnetic coupling of α-Fe2O3 nanoparticles

    NASA Astrophysics Data System (ADS)

    Frandsen, Cathrine; Mørup, Steen

    2006-08-01

    The magnetic properties of nanoparticles, including their superparamagnetic relaxation and spin orientation, have been found to depend on the aggregation state due to magnetic exchange coupling being established between surface atoms of neighbouring particles. We show that for samples of α-Fe2O3 nanoparticles the agglomeration and the interparticle exchange coupling are reversible processes. Grinding or ultrasonic treatment of aggregated particles can disperse the particles and reduce the magnetic coupling, while drying aqueous suspensions of dispersed particles leads to aggregation and re-establishment of magnetic coupling. The establishment of exchange coupling between neighbouring particles gives evidence for overlapping electronic orbitals of surface atoms of neighbouring particles. This is important not only for understanding the magnetic properties but also for understanding other physical properties e.g. the mechanical properties of dried aggregates. The reversibility (and the decoupling of particles) provides information on the strength of the coupling.

  17. Magnetization reversal mechanism of a sintered Nd-Fe-B magnet with Dy segregation

    SciTech Connect

    Suzuki, Hiroyuki; Satsu, Yuichi; Komuro, Matahiro; Kohashi, Teruo; Motai, Kumi

    2011-04-01

    The magnetization reversal mechanism of a sintered Nd-Fe-B magnet with Dy segregation near grain boundaries (GB) was studied using spin polarized scanning electron spectroscopy and magnetization measurements. More fine magnetic domains near GB were found in the magnet with Dy segregation than in the magnet without treatment. Magnetic modifications near the GB had no effect on the magnetization development. The domain wall motion of a quasihard magnetic component in the magnet with Dy segregation was suppressed in comparison with those in the magnet without treatment; this could also be confirmed in the different behaviors of asymmetry components toward a magnetic field direction between both magnets. From analyzing the probability of rotating magnetization near the GB, the magnetization reversal of the magnet with Dy segregation was more difficult to produce than those of the magnet without treatment.

  18. Magnetization reversal modes in fourfold Co nano-wire systems

    NASA Astrophysics Data System (ADS)

    Blachowicz, T.; Ehrmann, A.

    2015-09-01

    Magnetic nano-wire systems are, as well as other patterned magnetic structures, of special interest for novel applications, such as magnetic storage media. In these systems, the coupling between neighbouring magnetic units is most important for the magnetization reversal process of the complete system, leading to a variety of magnetization reversal mechanisms. This article examines the influence of the magnetic material on hysteresis loop shape, coercive field, and magnetization reversal modes. While iron nano-wire systems exhibit flat or one-step hysteresis loops, systems consisting of cobalt nano-wires show hysteresis loops with several longitudinal steps and transverse peaks, correlated to a rich spectrum of magnetization reversal mechanisms. We show that changing the material parameters while the system geometry stays identical can lead to completely different hysteresis loops and reversal modes. Thus, especially for finding magnetic nano-systems which can be used as quaternary or even higher-order storage devices, it is rational to test several materials for the planned systems. Apparently, new materials may lead to novel and unexpected behaviour - and can thus result in novel functionalities.

  19. Electrical detection of microwave assisted magnetization reversal by spin pumping

    SciTech Connect

    Rao, Siddharth; Subhra Mukherjee, Sankha; Elyasi, Mehrdad; Singh Bhatia, Charanjit; Yang, Hyunsoo

    2014-03-24

    Microwave assisted magnetization reversal has been investigated in a bilayer system of Pt/ferromagnet by detecting a change in the polarity of the spin pumping signal. The reversal process is studied in two material systems, Pt/CoFeB and Pt/NiFe, for different aspect ratios. The onset of the switching behavior is indicated by a sharp transition in the spin pumping voltage. At a threshold value of the external field, the switching process changes from partial to full reversal with increasing microwave power. The proposed method provides a simple way to detect microwave assisted magnetization reversal.

  20. Magnetic force microscopy investigation of the magnetization reversal of permalloy particles at high temperatures

    NASA Astrophysics Data System (ADS)

    Nurgazizov, N. I.; Khanipov, T. F.; Bizyaev, D. A.; Bukharaev, A. A.; Chuklanov, A. P.

    2014-09-01

    The magnetization reversal of an array of permalloy particles formed by scanning probe lithography on the silicon dioxide surface has been investigated in the temperature range from room temperature to 800 K. Using scanning magnetic force microscopy and numerical calculations of the magnetic anisotropy field of a particle at different temperatures, it has been shown that an increase in the temperature leads to a decrease in the external magnetic field required to reverse the magnetization direction of the particle. From the obtained results, it has been concluded that the magnetization reversal of the studied particles is accompanied by the formation of an intermediate state with an inhomogeneous magnetization structure.

  1. Reversible electric-field control of magnetization at oxide interfaces.

    PubMed

    Cuellar, F A; Liu, Y H; Salafranca, J; Nemes, N; Iborra, E; Sanchez-Santolino, G; Varela, M; Garcia Hernandez, M; Freeland, J W; Zhernenkov, M; Fitzsimmons, M R; Okamoto, S; Pennycook, S J; Bibes, M; Barthélémy, A; te Velthuis, S G E; Sefrioui, Z; Leon, C; Santamaria, J

    2014-06-23

    Electric-field control of magnetism has remained a major challenge which would greatly impact data storage technology. Although progress in this direction has been recently achieved, reversible magnetization switching by an electric field requires the assistance of a bias magnetic field. Here we take advantage of the novel electronic phenomena emerging at interfaces between correlated oxides and demonstrate reversible, voltage-driven magnetization switching without magnetic field. Sandwiching a non-superconducting cuprate between two manganese oxide layers, we find a novel form of magnetoelectric coupling arising from the orbital reconstruction at the interface between interfacial Mn spins and localized states in the CuO2 planes. This results in a ferromagnetic coupling between the manganite layers that can be controlled by a voltage. Consequently, magnetic tunnel junctions can be electrically toggled between two magnetization states, and the corresponding spin-dependent resistance states, in the absence of a magnetic field.

  2. Reversible electric-field control of magnetization at oxide interfaces.

    PubMed

    Cuellar, F A; Liu, Y H; Salafranca, J; Nemes, N; Iborra, E; Sanchez-Santolino, G; Varela, M; Garcia Hernandez, M; Freeland, J W; Zhernenkov, M; Fitzsimmons, M R; Okamoto, S; Pennycook, S J; Bibes, M; Barthélémy, A; te Velthuis, S G E; Sefrioui, Z; Leon, C; Santamaria, J

    2014-01-01

    Electric-field control of magnetism has remained a major challenge which would greatly impact data storage technology. Although progress in this direction has been recently achieved, reversible magnetization switching by an electric field requires the assistance of a bias magnetic field. Here we take advantage of the novel electronic phenomena emerging at interfaces between correlated oxides and demonstrate reversible, voltage-driven magnetization switching without magnetic field. Sandwiching a non-superconducting cuprate between two manganese oxide layers, we find a novel form of magnetoelectric coupling arising from the orbital reconstruction at the interface between interfacial Mn spins and localized states in the CuO2 planes. This results in a ferromagnetic coupling between the manganite layers that can be controlled by a voltage. Consequently, magnetic tunnel junctions can be electrically toggled between two magnetization states, and the corresponding spin-dependent resistance states, in the absence of a magnetic field. PMID:24953219

  3. Reverse draining of a magnetic soap film

    NASA Astrophysics Data System (ADS)

    Moulton, D. E.; Pelesko, J. A.

    2010-04-01

    We investigate the draining of a vertical magnetic soap film in the presence of a strong, nonuniform magnetic field. A colloidal suspension of magnetic nanoparticles in a regular soap solution yields a magnetic soap solution, from which a soap film is formed across an isolated frame. Experiments demonstrate that with a strong magnet placed above the frame, the film may be made to flow upward against gravity. The amount of film draining upward is altered by varying the distance between the frame and magnet. A first mathematical model is developed for the evolution of the film. Simulations demonstrate qualitative agreement with the experiment.

  4. A study on dynamic heat assisted magnetization reversal mechanisms under insufficient reversal field conditions

    SciTech Connect

    Chen, Y. J.; Yang, H. Z.; Leong, S. H.; Yu Ko, Hnin Yu; Wu, B. L.; Ng, V.; Asbahi, M.; Yang, J. K. W.

    2014-10-20

    We report an experimental study on the dynamic thermomagnetic (TM) reversal mechanisms at around Curie temperature (Tc) for isolated 60 nm pitch single-domain [Co/Pd] islands heated by a 1.5 μm spot size laser pulse under an applied magnetic reversal field (Hr). Magnetic force microscopy (MFM) observations with high resolution MFM tips clearly showed randomly trapped non-switched islands within the laser irradiated spot after dynamic TM reversal process with insufficient Hr strength. This observation provides direct experimental evidence by MFM of a large magnetization switching variation due to increased thermal fluctuation/agitation over magnetization energy at the elevated temperature of around Tc. The average percentage of non-switched islands/magnetization was further found to be inversely proportional to the applied reversal field Hr for incomplete magnetization reversal when Hr is less than 13% of the island coercivity (Hc), showing an increased switching field distribution (SFD) at elevated temperature of around Tc (where main contributions to SFD broadening are from Tc distribution and stronger thermal fluctuations). Our experimental study and results provide better understanding and insight on practical heat assisted magnetic recording (HAMR) process and recording performance, including HAMR writing magnetization dynamics induced SFD as well as associated DC saturation noise that limits areal density, as were previously observed and investigated by theoretical simulations.

  5. A study on dynamic heat assisted magnetization reversal mechanisms under insufficient reversal field conditions

    NASA Astrophysics Data System (ADS)

    Chen, Y. J.; Yang, H. Z.; Leong, S. H.; Wu, B. L.; Asbahi, M.; Yu Ko, Hnin Yu; Yang, J. K. W.; Ng, V.

    2014-10-01

    We report an experimental study on the dynamic thermomagnetic (TM) reversal mechanisms at around Curie temperature (Tc) for isolated 60 nm pitch single-domain [Co/Pd] islands heated by a 1.5 μm spot size laser pulse under an applied magnetic reversal field (Hr). Magnetic force microscopy (MFM) observations with high resolution MFM tips clearly showed randomly trapped non-switched islands within the laser irradiated spot after dynamic TM reversal process with insufficient Hr strength. This observation provides direct experimental evidence by MFM of a large magnetization switching variation due to increased thermal fluctuation/agitation over magnetization energy at the elevated temperature of around Tc. The average percentage of non-switched islands/magnetization was further found to be inversely proportional to the applied reversal field Hr for incomplete magnetization reversal when Hr is less than 13% of the island coercivity (Hc), showing an increased switching field distribution (SFD) at elevated temperature of around Tc (where main contributions to SFD broadening are from Tc distribution and stronger thermal fluctuations). Our experimental study and results provide better understanding and insight on practical heat assisted magnetic recording (HAMR) process and recording performance, including HAMR writing magnetization dynamics induced SFD as well as associated DC saturation noise that limits areal density, as were previously observed and investigated by theoretical simulations.

  6. Angular-dependent magnetization reversal processes in artificial spin ice

    NASA Astrophysics Data System (ADS)

    Burn, D. M.; Chadha, M.; Branford, W. R.

    2015-12-01

    The angular dependence of the magnetization reversal in interconnected kagome artificial spin ice structures has been studied through experimental MOKE measurements and micromagnetic simulations. This reversal is mediated by the propagation of magnetic domain walls along the interconnecting bars, which either nucleate at the vertex or arrive following an interaction in a neighboring vertex. The physical differences in these processes show a distinct angular dependence allowing the different contributions to be identified. The configuration of the initial magnetization state, either locally or on a full sublattice of the system, controls the reversal characteristics of the array within a certain field window. This shows how the available magnetization reversal routes can be manipulated and the system can be trained.

  7. Magnetization reversal in melt-quenched NdFeB

    SciTech Connect

    Crew, D.C.; Lewis, L.H.; McCormick, P.G.; Street, R.; Panchanathan, V.

    1999-06-01

    Melt-quenched NdFeB is an important modern permanent magnet material. However there still remains doubt as to the magnetization reversal mechanism which controls coercivity in material prepared by this processing route. To investigate this problem a new technique based on measurements of reversible magnetization along recoil curves has been used. The technique identifies the presence of free domain walls during magnetic reversal. For this study samples of isotropic (MQI), hot pressed (MQII) and die upset (MQIII) melt-quenched NdFeB were examined. The results indicate that in MQI free domain walls are not present during reversal and the reversal mechanism is most likely incoherent rotation of some form. Free domain walls are also not present during reversal in the majority of grains of MQII, even though initial magnetization measurements indicate that the grain size is large enough to support them. In MQIII free domain walls are present during reversal. These results are attributed to the reduced domain wall nucleation field in MQIII compared with MQII and the increased dipolar interactions in MQIII.

  8. Magnetic field evolution and reversals in spiral galaxies

    NASA Astrophysics Data System (ADS)

    Dobbs, C. L.; Price, D. J.; Pettitt, A. R.; Bate, M. R.; Tricco, T. S.

    2016-10-01

    We study the evolution of galactic magnetic fields using 3D smoothed particle magnetohydrodynamics (SPMHD) simulations of galaxies with an imposed spiral potential. We consider the appearance of reversals of the field, and amplification of the field. We find that magnetic field reversals occur when the velocity jump across the spiral shock is above ≈20 km s-1, occurring where the velocity change is highest, typically at the inner Lindblad resonance in our models. Reversals also occur at corotation, where the direction of the velocity field reverses in the corotating frame of a spiral arm. They occur earlier with a stronger amplitude spiral potential, and later or not at all with weaker or no spiral arms. The presence of a reversal at radii of around 4-6 kpc in our fiducial model is consistent with a reversal identified in the Milky Way, though we caution that alternative Galaxy models could give a similar reversal. We find that relatively high resolution, a few million particles in SPMHD, is required to produce consistent behaviour of the magnetic field. Amplification of the magnetic field occurs in the models, and while some may be genuinely attributable to differential rotation or spiral arms, some may be a numerical artefact. We check our results using ATHENA, finding reversals but less amplification of the field, suggesting that some of the amplification of the field with SPMHD is numerical.

  9. Spin reversal in Fe8 under fast pulsed magnetic fields

    NASA Astrophysics Data System (ADS)

    Narayana Jammalamadaka, S.; Vélez, S.; Vanacken, J.; Moshchalkov, V. V.; Chibotaru, L. F.; Tejada, J.; Macià, F.

    2015-07-01

    We report measurements on magnetization reversal in the Fe8 molecular magnet using fast pulsed magnetic fields of 1.5 kT s-1 and in the temperature range of 0.6-4.1 K. We observe and analyze the temperature dependence of the reversal process, which involves in some cases several resonances. Our experiments allow observation of resonant quantum tunneling of magnetization up to a temperature of ˜4 K. We also observe shifts in the maxima of the relaxation within each resonance field with temperature that suggest the emergence of a thermal instability—a combination of spin reversal and self-heating that may result in a magnetic deflagration process. The results are mainly understood in the framework of thermally-activated quantum tunneling transitions in combination with emergence of a thermal instability.

  10. Dipolar energy of Nd-Fe-B nanocrystalline magnets in magnetization reversal process

    NASA Astrophysics Data System (ADS)

    Ohtori, Hiroyuki; Iwano, Kaoru; Mitsumata, Chiharu; Yano, Masao; Kato, Akira; Shoji, Tetsuya; Manabe, Akira; Ono, Kanta

    2014-05-01

    We analyzed the dipolar energy of Nd-Fe-B nanocrystalline magnets in magnetization reversal process through visualizing magnetic dipolar interaction. We obtained magnetization distribution images experimentally by using scanning transmission X-ray microscopy (STXM). The magnetic dipolar interaction was calculated by the interaction between the magnetization at each point and those at the other points on the STXM image. We showed the dipolar energy in the nanocrystalline Nd-Fe-B magnets and compared it with the exchange energy at various applied fields. Our results indicated the significance of the dipolar energy in magnetization reversal process.

  11. Particle Dynamics Discrimination Between Current Sheet Magnetic Field Reversal and Magnetic Neutral Line Fields

    NASA Astrophysics Data System (ADS)

    Martin, R. F., Jr.; Holland, D. L.; Svetich, J.

    2014-12-01

    We consider dynamical signatures of ion motion that discriminate between a current sheet magnetic field reversal and a magnetic neutral line field. These two related dynamical systems have been studied previously as chaotic scattering systems with application to the Earth's magnetotail. Both systems exhibit chaotic scattering over a wide range of parameter values. The structure and properties of their respective phase spaces have been used to elucidate potential dynamical signatures that affect spacecraft measured ion distributions. In this work we consider the problem of discrimination between these two magnetic structures using charged particle dynamics. For example we show that signatures based on the well known energy resonance in the current sheet field provide good discrimination since the resonance is not present in the neutral line case. While both fields can lead to fractal exit region structuring, their characteristics are different and also may provide some field discrimination. Application to magnetotail field and particle parameters will be presented

  12. Fast chirality reversal of the magnetic vortex by electric current

    SciTech Connect

    Lim, W. L. Liu, R. H.; Urazhdin, S.; Tyliszczak, T.; Erokhin, S. G.; Berkov, D.

    2014-12-01

    The possibility of high-density information encoding in magnetic materials by topologically stable inhomogeneous magnetization configurations such as domain walls, skyrmions, and vortices has motivated intense research into mechanisms enabling their control and detection. While the uniform magnetization states can be efficiently controlled by electric current using magnetic multilayer structures, this approach has proven much more difficult to implement for inhomogeneous states. Here, we report direct observation of fast reversal of magnetic vortex by electric current in a simple planar structure based on a bilayer of spin Hall material Pt with a single microscopic ferromagnetic disk contacted by asymmetric electrodes. The reversal is enabled by a combination of the chiral Oersted field and spin current generated by the nonuniform current distribution in Pt. Our results provide a route for the efficient control of inhomogeneous magnetization configurations by electric current.

  13. Magnetic Properties of Nanostructures

    NASA Astrophysics Data System (ADS)

    Ciraldo, John

    2007-10-01

    The recent development of the superlattice nanowire pattern transfer (SNAP) technique has enabled the fabrication of complex molecular-electronic circuits at unprecedented densities. In this project, we explore the possibility of extending this technique to generate comparably dense arrays of nanoscale giant magnetoresistive (GMR) and tunneling magnetoresistive (TMR) devices. My primary contribution to this project has focused on using a vibrating sample magnetometer (VSM), as well as a superconducting interference device (SQUID) magnetometer to monitor the magnetic properties of the devices as they are processed from thin 2D films into nanostructure arrays. This investigation allows us to investigate both fundamental and technological aspects of the nanopatterning process. For example, the effects of changing surface to volume ratios on the ferromagnetic exchange interaction and the role of various patterning techniques in determining surface chemistry and oxidation of the final nanostructures, respectively. Additionally I have worked on simulations of the materials using NIST's OOMF program, allowing me to compare actual results with theoretical expectations. I am also designing a magneto-optical Kerr effect (MOKE) detector, which will allow faster approximations of magnetic behavior.

  14. Magnetic flux trapping during field reversal in the formation of a field-reversed configuration

    NASA Astrophysics Data System (ADS)

    Steinhauer, Loren C.

    1985-11-01

    The flow of plasma and magnetic flux toward a wall is examined in a slab geometry where the magnetic field is parallel to the wall. Magnetohydrodynamic (MHD) flow with a quasisteady approximation is assumed that reduces the problem to three coupled ordinary differential equations. The calculated behavior shows that a thin current sheath is established at the wall in which a variety of phenomena appear, including significant resistive heating and rapid deceleration of the plasma flow. The sheath physics determines the speed at which flux and plasma flow toward the wall. The model has been applied to the field-reversal phase of a field-reversed theta pinch, during which the reduced magnetic field near the wall drives an outward flow of plasma and magnetic flux. The analysis leads to approximate expressions for the instantaneous flow speed, the loss of magnetic flux during the field reversal phase, the integrated heat flow to the wall, and the highest possible magnetic flux retained after reversal. Predictions from this model are compared with previous time-dependent MHD calculations and with experimental results from the TRX-1 [Proceedings of the 4th Symposium on the Physics and Technology of Compact Toroids, 27-29 October 1981 (Lawrence Livermore National Laboratory, Livermore, CA, 1982), p. 61] and TRX-2 [Proceedings of the 6th U.S. Symposium on Compact Toroid Research, 20-23 February, 1984 (Princeton Plasma Physics Laboratory, Princeton, NJ, 1984), p. 154] experiments.

  15. Magnetization Reversal Processes, in the Nanocrystalline Fe-Co-Zr-Ti-Pr-B Magnets

    NASA Astrophysics Data System (ADS)

    Pawlik, K.; Pawlik, P.; Wysłocki, J. J.; Kaszuwara, W.

    2008-01-01

    Magnetization reversal processes in the magnets derived from the Fe60Co13Zr1Ti3Pr9B14 alloy were investigated. It was shown that the processing technique affects the magnetization reversal processes. For the nanocrystalline ribbon samples pinning of the domain walls arises at low external magnetic fields while nucleation of reversed domains occurs at higher fields. However, the nucleation fields are lower than the pinning fields for the nanocrystalline rod and tube samples produced by suction-casting technique.

  16. Magnetization reversal in cobalt and nickel electrodeposited nanowires

    NASA Astrophysics Data System (ADS)

    Ounadjela, K.; Ferré, R.; Louail, L.; George, J. M.; Maurice, J. L.; Piraux, L.; Dubois, S.

    1997-04-01

    We have investigated the magnetization reversal processes in arrays of sub-micron Ni and Co wires by means of magnetization and torque experiments together with micromagnetic calculations. The wires were produced by electrodeposition in the cylindrical pores of track-etched polymer membranes. Diameters in the range 35-400 nm have been studied. The arrays of Co and Ni nanowires display different magnetic behaviors. Particular emphasis is given to the competing shape and crystal magnetic anisotropies that exist in the Co nanowire system. In both systems, explaining the experimental results requires domain formation, except for the smallest diameters where single domain behavior occurs.

  17. All-optical magnetization reversal by circularly polarized laser pulses: Experiment and multiscale modeling

    NASA Astrophysics Data System (ADS)

    Vahaplar, K.; Kalashnikova, A. M.; Kimel, A. V.; Gerlach, S.; Hinzke, D.; Nowak, U.; Chantrell, R.; Tsukamoto, A.; Itoh, A.; Kirilyuk, A.; Rasing, Th.

    2012-03-01

    We present results of detailed experimental and theoretical studies of all-optical magnetization reversal by single circularly-polarized laser pulses in ferrimagnetic rare earth—transition metal (RE-TM) alloys GdxFe90-xCo10 (20%magnetization during the reversal process. This reversal does not involve precessional motion of magnetization but is governed by the longitudinal relaxation and thus has a linear character. We demonstrate that this all-optically driven linear reversal can be modeled as a result of a two-fold impact of the laser pulse on the medium. First, due to absorption of the light and ultrafast laser-induced heating, the medium is brought to a highly nonequilibrium state. Simultaneously, due to the ultrafast inverse Faraday effect the circularly polarized laser pulse acts as an effective magnetic field of the amplitude up to ˜20 T. We show that the polarization-dependent reversal triggered by the circularly polarized light is feasible only in a narrow range (below 10%) of laser fluences. The duration of the laser pulse required for the reversal can be varied from ˜40 fs up to at least ˜1700 fs. We also investigate experimentally the role of the ferrimagnetic properties of GdFeCo in the all-optical reversal. In particular, the optimal conditions for the all-optical reversal are achieved just below the ferrimagnetic compensation temperature, where the magnetic information can be all-optically written by a laser pulse of minimal fluence and read out within just 30 ps. We argue that this is the fastest write-read event demonstrated for magnetic recording so far.

  18. Electrical detection of magnetization reversal without auxiliary magnets

    NASA Astrophysics Data System (ADS)

    Olejník, K.; Novák, V.; Wunderlich, J.; Jungwirth, T.

    2015-05-01

    First-generation magnetic random access memories based on anisotropic magnetoresistance required magnetic fields for both writing and reading. Modern all-electrical read/write memories use instead nonrelativistic spin transport connecting the storing magnetic layer with a reference ferromagnet. Recent studies have focused on electrical manipulation of magnetic moments by relativistic spin torques requiring no reference ferromagnet. Here we report the observation of a counterpart magnetoresistance effect in such a relativistic system which allows us to electrically detect the sign of the magnetization without an auxiliary magnetic field or ferromagnet. We observe the effect in a geometry in which the magnetization of a uniaxial (Ga,Mn)As epilayer is set either parallel or antiparallel to a current-induced nonequilibrium spin polarization of carriers. In our structure, this linear-in-current magnetoresistance reaches 0.2% at current density of 106Acm -2 .

  19. Field orientation dependence of magnetization reversal in thin films with perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Fallarino, Lorenzo; Hovorka, Ondrej; Berger, Andreas

    2016-08-01

    The magnetization reversal process of hexagonal-close-packed (hcp) (0001) oriented Co and C o90R u10 thin films with perpendicular magnetic anisotropy (PMA) has been studied as a function of temperature and applied magnetic field angle. Room temperature pure cobalt exhibits two characteristic reversal mechanisms. For angles near in-plane field orientation, the magnetization reversal proceeds via instability of the uniform magnetic state, whereas in the vicinity of the out-of-plane (OP) orientation, magnetization inversion takes place by means of domain nucleation. Temperature dependent measurements enable the modification of the magnetocrystalline anisotropy and reveal a gradual disappearance of the domain nucleation process during magnetization reversal for elevated temperatures. Ultimately, this suppression of the domain nucleation process leads to the exclusive occurrence of uniform state instability reversal for all field orientations at sufficiently high temperature. Comparative magnetic measurements of C o90R u10 alloy samples allow the identification and confirmation of the high temperature remanent magnetization state of cobalt as an OP stripe domain state despite the reduction of magnetocrystalline anisotropy. Detailed micromagnetic simulations supplement the experimental results and corroborate the physical understanding of the temperature dependent behavior. Moreover, they enable a comprehensive identification of the complex energy balance in magnetic films with PMA, for which three different magnetic phases occur for sufficiently high anisotropy values, whose coexistence point is tricritical in nature.

  20. Magnetic field reversals: the geodynamo, laboratory experiments and models (Lewis Fry Richardson Medal Lecture)

    NASA Astrophysics Data System (ADS)

    Fauve, S.

    2009-04-01

    I will first compare reversals of Earth's magnetic field known from palaeomagnetic data to the ones observed in a laboratory experiment for the magnetic field generated by a turbulent flow of liquid sodium (VKS experiment). Despite major differences between the flow in Earth's core and in the experiment, both systems display reversals that share a lot of similar properties. I will understand them using a simple model in the framework of low dynamical system theory. Finally, I will discuss what can be learnt from numerical simulations.

  1. Experimental study of magnetization reversal processes in nonsymmetric spin valve

    NASA Astrophysics Data System (ADS)

    Gornakov, V. S.; Nikitenko, V. I.; Bennett, L. H.; Brown, H. J.; Donahue, M. J.; Egelhoff, W. F.; McMichael, R. D.; Shapiro, A. J.

    1997-04-01

    We have investigated a nonsymmetric bottom giant magnetoresistance spin valve with the structure Si/NiO/Co/Cu/Co/Ta, as well as single ferromagnetic Co layers on antiferromagnetic NiO, with or without a nonmagnetic Cu spacer. Magnetic hysteresis loops have been measured by SQUID magnetometry, and magnetic domain structures have been imaged using an advanced magneto-optical indicator film (MOIF) technique. The MOIF technique demonstrated that the first stage of magnetization reversal is characterized by nucleation of many microdomains. With increasing reversed field, the domain walls move over small distances (5-20 μm) until annihilation. The domain size was observed to increase with the thickness of the Co layer. When an alternating magnetic field was applied, the domain structure was dramatically changed.

  2. Thermal effects on the magnetization reversal process and its interpretation in perpendicular magnetic recording media

    NASA Astrophysics Data System (ADS)

    Srinivasan, Kumar; Acharya, B. Ramamurthy; Bertero, Gerardo

    2010-06-01

    We have studied the time-scale and temperature dependence of the magnetization reversal in perpendicular magnetic recording media. One of the under-reported phenomena associated with this reversal is the thermal dependence of the squareness of the magnetic hysteresis loop. Understanding this phenomenon is important because the coercive squareness parameter S∗ is often used to evaluate the strength of the magnetic exchange-coupling interactions between the grains. In this work, we demonstrate that S∗ is a dynamic quantity which depends on the thermal agitation of the magnetization, and it is imperative to take this dependence into account in interpreting magnetic and microstructural effects. Based on the Sharrock model for the dynamic coercivity, we built an expression for the time-scale and temperature dependence of S∗ in highly oriented perpendicular magnetic recording media. Fits of experimental data to the resulting expression were then used to extract the intrinsic squareness parameter Sint∗ which originates in the thermal-independent demagnetization and exchange-interaction effects. Sint∗ was estimated for two sets of perpendicular recording media samples. For the first set of media samples showing progressively smaller grain sizes, the values of S∗ measured at the normal magnetometry time-scales of milliseconds to seconds indicated progressively smaller values. In contrast, the values of the thermal-independent S∗ determined from applying the above model were progressively larger. This discrepancy can only be explained on the basis of progressively stronger intergranular exchange coupling, which is offset by strong thermal effects at small grain sizes. For the second set of media samples with increasingly larger segregant oxide content, progressively smaller values of both S∗ and thermal-independent Sint∗ were observed, thus verifying the strong intergranular segregation effects due to greater nonmagnetic grain boundary phase. The

  3. Magnetization reversal in orthogonal spin transfer magnetic devices

    NASA Astrophysics Data System (ADS)

    Wolf, Georg; Kent, Andrew D.; Kardasz, Bartek; Pinarbasi, Mustafa

    2014-03-01

    Orthogonal spin transfer (OST) magnetic devices have distinct magnetization dynamics and switching characteristics compared to conventional collinearly magnetized devices. A perpendicular magnetized layer provides a large initial spin torque on the free layer magnetization and thus initiates magnetization dynamics. In order to read out the information stored in the OST device, the free layer forms a magnetic tunnel junction with an in plane magnetized reference layer, which also exerts a spin torque on the free layer. The combination of those two spin torques leads to different switching dynamics of the free layer. Quasistatic and fast pulsed measurements have been conducted to explore the state diagram and magnetization dynamics of such devices. The absolute value of the switching current Is is in general smaller for the antiparallel (AP) to parallel (P) transition, due to the angular dependence of the reference layer torque. Is also has a weak field dependence for this transition, indicating that the reference layer torque governs this transition. On the other hand, the P to AP transition shows a stronger field dependence of Is and occurs for both current polarities. Both these features denote the influence of the spin-torque generated from the perpendicular polarizer. Supported by STT Inc.

  4. Paleomagnetic Study of a Reversal of the Earth's Magnetic Field.

    PubMed

    Dunn, J R; Fuller, M; Ito, H; Schmidt, V A

    1971-05-21

    A detailed record of a field reversal has been obtained from the natural remanent magnetization of the Tatoosh intrusion in Mount Rainier National Park, Washington. The reversal took place at 14.7 +/- 1 million years and is interpreted to be from reverse to normal. A decrease in the intensity of the field of about an order of magnitude occurs immediately before the reversal, while its orientation remains substantially unchanged. The onset of the reversal is marked by abrupt swinging of the virtual geomagnetic pole along an arc of a great circle. During the reversal the pole traces a path across the Pacific. In the last stage of the process recorded in the sections, the succession of virtual geomagnetic poles is very similar to those generated by secular variation in the recent past. Although the cooling rate of the intrusion is not sufficiently well known to permit a useful calculation of the duration of the reversal process, an estimate based on the length of the supposed secular variation cycles gives 1 to 4 x 103 years for the reversal of field direction and approximately 1 x 104 years for the time scale of the intensity changes. PMID:17792941

  5. Control over magnetic properties in bulk hybrid materials

    NASA Astrophysics Data System (ADS)

    Urban, Christian; Quesada, Adrian; Saerbeck, Thomas; Rubia, Miguel Angel De La; Garcia, Miguel Angel; Fernandez, Jose Francisco; Schuller, Ivan K.; UCSD Collaboration; Instituto de Ceramica, Madrid Collaboration; Institut Laue-Langevin, Grenoble Collaboration

    We present control of coercivity and remanent magnetization of a bulk ferromagnetic material embedded in bulk vanadium sesquioxide (V2O3) by using a standard bulk synthesis procedure. The method generalizes the use of structural phase transitions of one material to control structural and magnetic properties of another. A structural phase transition (SPT) in the V2O3 host material causes magnetic properties of Ni to change as function of temperature. The remanent magnetization and the coercivity are reversibly controlled by the SPT without additional external magnetic fields. The reversible tuning shown here opens the pathway for controlling the properties of a vast variety of magnetic hybrid bulk systems. This Work is supported by the Office of Basic Energy Science, U.S. Department of Energy, BES-DMS funded by the Department of Energy's Office of Basic Energy Science, DMR under grant DE FG02 87ER-45332.

  6. Self-reversal and apparent magnetic excursions in Arctic sediments

    NASA Astrophysics Data System (ADS)

    Channell, J. E. T.; Xuan, C.

    2009-06-01

    The Arctic oceans have been fertile ground for the recording of apparent excursions of the geomagnetic field, implying that the high latitude field had unusual characteristics at least over the last 1-2 Myrs. Alternating field demagnetization of the natural remanent magnetization (NRM) of Core HLY0503-6JPC from the Mendeleev Ridge (Arctic Ocean) implies the presence of primary magnetizations with negative inclination apparently recording excursions in sediments deposited during the Brunhes Chron. Thermal demagnetization, on the other hand, indicates the presence of multiple (often anti-parallel) magnetization components with negative inclination components having blocking temperatures predominantly, but not entirely, below ~ 350 °C. Thermo-magnetic tests, X-ray diffraction (XRD) and scanning electron microscopy (SEM) indicate that the negative inclination components are carried by titanomaghemite, presumably formed by seafloor oxidation of titanomagnetite. The titanomaghemite apparently carries a chemical remanent magnetization (CRM) that is partially self-reversed relative to the detrital remanent magnetization (DRM) carried by the host titanomagnetite. The partial self-reversal could have been accomplished by ionic ordering during oxidation, thereby changing the balance of the magnetic moments in the ferrimagnetic sublattices.

  7. Magnetization reversal of an individual exchange-biased permalloy nanotube

    NASA Astrophysics Data System (ADS)

    Buchter, A.; Wölbing, R.; Wyss, M.; Kieler, O. F.; Weimann, T.; Kohlmann, J.; Zorin, A. B.; Rüffer, D.; Matteini, F.; Tütüncüoglu, G.; Heimbach, F.; Kleibert, A.; Fontcuberta i Morral, A.; Grundler, D.; Kleiner, R.; Koelle, D.; Poggio, M.

    2015-12-01

    We investigate the magnetization reversal mechanism in an individual permalloy (Py) nanotube (NT) using a hybrid magnetometer consisting of a nanometer-scale SQUID (nanoSQUID) and a cantilever torque sensor. The Py NT is affixed to the tip of a Si cantilever and positioned in order to optimally couple its stray flux into a Nb nanoSQUID. We are thus able to measure both the NT's volume magnetization by dynamic cantilever magnetometry and its stray flux using the nanoSQUID. We observe a training effect and a temperature dependence in the magnetic hysteresis, suggesting an exchange bias. We find a low blocking temperature TB=18 ±2 K, indicating the presence of a thin antiferromagnetic native oxide, as confirmed by x-ray absorption spectroscopy on similar samples. Furthermore, we measure changes in the shape of the magnetic hysteresis as a function of temperature and increased training. These observations show that the presence of a thin exchange-coupled native oxide modifies the magnetization reversal process at low temperatures. Complementary information obtained via cantilever and nanoSQUID magnetometry allows us to conclude that, in the absence of exchange coupling, this reversal process is nucleated at the NT's ends and propagates along its length as predicted by theory.

  8. Investigation of the magnetization reversal mechanism of electrolessly deposited Co-B nanotubes

    NASA Astrophysics Data System (ADS)

    Richardson, David; Kingston, Samuel; Rhen, Fernando M. F.

    2016-05-01

    Co-B nanotubes were prepared via an electroless deposition method. The morphology, magnetic properties and the magnetization reversal mechanism of the nanotubes were investigated. Deposition was carried out in porous polycarbonate membranes leading to the formation of Co-B nanotubes with an average external diameter of 400 nm and lengths up to 6 μm. Electroless deposition resulted in the formation of alloys with composition Co70B30 and a specific magnetization of 65.6 J T-1kg-1, which is about 40 % of that of pure Co (161 J T-1kg-1). The transversal and vortex modes were identified as the mechanisms responsible for magnetization reversal in the nanotubes. A crossover between the two modes is observed at low angles and the results are in line with current models for switching mechanisms of nanotubes.

  9. Magnetization and microstructure dynamics in Fe/MnAs/GaAs(001): Fe magnetization reversal by a femtosecond laser pulse.

    PubMed

    Spezzani, C; Ferrari, E; Allaria, E; Vidal, F; Ciavardini, A; Delaunay, R; Capotondi, F; Pedersoli, E; Coreno, M; Svetina, C; Raimondi, L; Zangrando, M; Ivanov, R; Nikolov, I; Demidovich, A; Danailov, M B; Popescu, H; Eddrief, M; De Ninno, G; Kiskinova, M; Sacchi, M

    2014-12-12

    Thin film magnetization reversal without applying external fields is an attractive perspective for applications in sensors and devices. One way to accomplish it is by fine-tuning the microstructure of a magnetic substrate via temperature control, as in the case of a thin Fe layer deposited on a MnAs/GaAs(001) template. This work reports a time-resolved resonant scattering study exploring the magnetic and structural properties of the Fe/MnAs system, using a 100 fs optical laser pulse to trigger local temperature variations and a 100 fs x-ray free-electron laser pulse to probe the induced magnetic and structural dynamics. The experiment provides direct evidence that a single optical laser pulse can reverse the Fe magnetization locally. It reveals that the time scale of the magnetization reversal is slower than that of the MnAs structural transformations triggered by the optical pulse, which take place after a few picoseconds already.

  10. Voltage controlled core reversal of fixed magnetic skyrmions without a magnetic field

    NASA Astrophysics Data System (ADS)

    Bhattacharya, Dhritiman; Al-Rashid, Md Mamun; Atulasimha, Jayasimha

    2016-08-01

    Using micromagnetic simulations we demonstrate core reversal of a fixed magnetic skyrmion by modulating the perpendicular magnetic anisotropy of a nanomagnet with an electric field. We can switch reversibly between two skyrmion states and two ferromagnetic states, i.e. skyrmion states with the magnetization of the core pointing down/up and periphery pointing up/down, and ferromagnetic states with magnetization pointing up/down, by sequential increase and decrease of the perpendicular magnetic anisotropy. The switching between these states is explained by the fact that the spin texture corresponding to each of these stable states minimizes the sum of the magnetic anisotropy, demagnetization, Dzyaloshinskii-Moriya interaction (DMI) and exchange energies. This could lead to the possibility of energy efficient nanomagnetic memory and logic devices implemented with fixed skyrmions without using a magnetic field and without moving skyrmions with a current.

  11. Voltage controlled core reversal of fixed magnetic skyrmions without a magnetic field.

    PubMed

    Bhattacharya, Dhritiman; Al-Rashid, Md Mamun; Atulasimha, Jayasimha

    2016-01-01

    Using micromagnetic simulations we demonstrate core reversal of a fixed magnetic skyrmion by modulating the perpendicular magnetic anisotropy of a nanomagnet with an electric field. We can switch reversibly between two skyrmion states and two ferromagnetic states, i.e. skyrmion states with the magnetization of the core pointing down/up and periphery pointing up/down, and ferromagnetic states with magnetization pointing up/down, by sequential increase and decrease of the perpendicular magnetic anisotropy. The switching between these states is explained by the fact that the spin texture corresponding to each of these stable states minimizes the sum of the magnetic anisotropy, demagnetization, Dzyaloshinskii-Moriya interaction (DMI) and exchange energies. This could lead to the possibility of energy efficient nanomagnetic memory and logic devices implemented with fixed skyrmions without using a magnetic field and without moving skyrmions with a current. PMID:27506159

  12. Size and shape dependence study of magnetization reversal in magnetic antidot lattice arrays

    NASA Astrophysics Data System (ADS)

    Mallick, Sougata; Bedanta, Subhankar

    2015-05-01

    Magnetic Antidot Lattice (MAL) arrays of Co have been prepared in micron range using ultraviolet (UV) lithography technique with different shapes and sizes. Magnetization reversal in such MAL systems has been studied by magneto-optic Kerr effect (MOKE) based microscopy by varying the angle between the easy axis and the external magnetic field. The domain images evidence that the magnetization reversal along easy axis is highly dominated by nucleation of domains which is subsequently accompanied by domain wall motion. We have observed that with increase in active magnetic area domain size increases but on the contrary coercivity decreases. The presence of periodic holes turns the MALs magnetically hard when compared to similar thickness of continuous thin film. The magnetization relaxation along easy axis for the Co MAL at constant dc field fits very well with the exponential law of Fatuzzo-Labrune indicating domain nucleated dominant process.

  13. Voltage controlled core reversal of fixed magnetic skyrmions without a magnetic field

    PubMed Central

    Bhattacharya, Dhritiman; Al-Rashid, Md Mamun; Atulasimha, Jayasimha

    2016-01-01

    Using micromagnetic simulations we demonstrate core reversal of a fixed magnetic skyrmion by modulating the perpendicular magnetic anisotropy of a nanomagnet with an electric field. We can switch reversibly between two skyrmion states and two ferromagnetic states, i.e. skyrmion states with the magnetization of the core pointing down/up and periphery pointing up/down, and ferromagnetic states with magnetization pointing up/down, by sequential increase and decrease of the perpendicular magnetic anisotropy. The switching between these states is explained by the fact that the spin texture corresponding to each of these stable states minimizes the sum of the magnetic anisotropy, demagnetization, Dzyaloshinskii-Moriya interaction (DMI) and exchange energies. This could lead to the possibility of energy efficient nanomagnetic memory and logic devices implemented with fixed skyrmions without using a magnetic field and without moving skyrmions with a current. PMID:27506159

  14. Transition states of magnetization reversal in ferromagnetic nanorings

    NASA Astrophysics Data System (ADS)

    Chaves-O'Flynn, Gabriel; Kent, Andrew; Stein, Daniel

    2008-03-01

    Thin ferromagnetic rings are of interest for fundamental studies of magnetization reversal, in part, because they are a rare example of a geometry for which an analytical solution for the rate of thermally induced switching has been determined [1]. The theoretical model predicts the transition state to be either a global magnetization rotation of constant azimuthal angle or a localized fluctuation, denoted the instanton saddle. Numerically we have confirmed that for a range of values of external magnetic field and ring size the instanton saddle is energetically favored [2]. The model takes the annular width to be small compared to the mean radius of the annulus; in which case the main contribution to the magnetization energy comes from the surface magnetostatic energy. We present numerical micromagnetic calculations of the activation energy for thermally induced magnetization reversal for the two different transition states for the case when the annular width is equal in magnitude to the mean radius of the ring. Results of the total and surface magnetostatic energies are compared for different ring sizes. [1] K. Martens, D.L. Stein, A.D. Kent, PRB 73, 054413 (2006) [2] G.D. Chaves-O'Flynn, K. Xiao, D.L. Stein, A. D. Kent, arXiv:0710.2546 (2007)

  15. SOLAR MAGNETIC FIELD REVERSALS AND THE ROLE OF DYNAMO FAMILIES

    SciTech Connect

    DeRosa, M. L.

    2012-09-20

    The variable magnetic field of the solar photosphere exhibits periodic reversals as a result of dynamo activity occurring within the solar interior. We decompose the surface field as observed by both the Wilcox Solar Observatory and the Michelson Doppler Imager into its harmonic constituents, and present the time evolution of the mode coefficients for the past three sunspot cycles. The interplay between the various modes is then interpreted from the perspective of general dynamo theory, where the coupling between the primary and secondary families of modes is found to correlate with large-scale polarity reversals for many examples of cyclic dynamos. Mean-field dynamos based on the solar parameter regime are then used to explore how such couplings may result in the various long-term trends in the surface magnetic field observed to occur in the solar case.

  16. Magnetization reversal in magnetic dot arrays: Nearest-neighbor interactions and global configurational anisotropy

    NASA Astrophysics Data System (ADS)

    Van de Wiele, Ben; Fin, Samuele; Pancaldi, Matteo; Vavassori, Paolo; Sarella, Anandakumar; Bisero, Diego

    2016-05-01

    Various proposals for future magnetic memories, data processing devices, and sensors rely on a precise control of the magnetization ground state and magnetization reversal process in periodically patterned media. In finite dot arrays, such control is hampered by the magnetostatic interactions between the nanomagnets, leading to the non-uniform magnetization state distributions throughout the sample while reversing. In this paper, we evidence how during reversal typical geometric arrangements of dots in an identical magnetization state appear that originate in the dominance of either Global Configurational Anisotropy or Nearest-Neighbor Magnetostatic interactions, which depends on the fields at which the magnetization reversal sets in. Based on our findings, we propose design rules to obtain the uniform magnetization state distributions throughout the array, and also suggest future research directions to achieve non-uniform state distributions of interest, e.g., when aiming at guiding spin wave edge-modes through dot arrays. Our insights are based on the Magneto-Optical Kerr Effect and Magnetic Force Microscopy measurements as well as the extensive micromagnetic simulations.

  17. Centenary of the Discovery of Earth's Magnetic Field Reversals

    NASA Astrophysics Data System (ADS)

    Kornprobst, Jacques; Lénat, Jean-François

    2014-11-01

    In the early years of the 20th century, physicist Bernard Brunhes, then director of the Geophysical Observatory of Puy de Dôme (now Observatoire de Physique du Globe de Clermont), measured for the first time reverse magnetization in samples from a basaltic lava flow and from the underlying backed argillaceous sediments from the village of Pontfarein (now Pont Farin) in the Cantal volcanic district (Auvergne, France).

  18. Magnetic reversal spurts: Rain gauges for comet showers

    NASA Technical Reports Server (NTRS)

    Lutz, T. M.

    1988-01-01

    Abrupt increases in the rate of magnetic reversals (magnetic reversal spurts) were first studied by many others. They hypothesized that spurts result from increased turbulence in the earth's core dynamo during episodes of intense bolide bombardment of the earth. Mechanisms for creating episodes of intense bombardment of the earth involve gravitational perturbation of the Oort cloud of comets, either by a hidden planet, a solar companion, or massive matter in the galactic plane. Herein, the time variation in reversal rate is analyzed using methods of statistical density estimation. A smooth, continuous estimate of reversal rate is obtained using an adaptive kernel method, in which the kernel width is adjusted as a function of reversal rate. The estimates near the ends of the data series (at 165 my ago and the present) are obtained by extending the data by reflection. The results show that the reversal spurts are not associated demonstrably with extinctions or well-dated impacts. If the spurts do record episodes of intense bombardment of the earth, then the mass extinctions do not, in general, occur at times of impacts. Furthermore, the large impact craters seen are not obviously related to the spurts, suggesting that the craters may have been caused by bolides of a different nature and with a different temporal pattern. However, the most simple explanation seems to be that the spurts do not record comet showers, either because the recording mechanism suggested by Muller and Morris is not effective or because comet showers are not triggered in the ways considered by Hut et al.

  19. Magnetically induced enhancement of reversibly responding conductometric sensors

    SciTech Connect

    Baker, Caitlin; Laminack, William; Tune, Travis; Gole, James

    2014-04-28

    Small magnetic fields are found to greatly enhance the reversible room temperature conductometric responses of n and p- type porous silicon (PS) interfaces, treated with nanostructured island sites containing paramagnetic Co(II) and Fe(II). At concentrations sufficiently low so as to avoid cross talk between the nanostructured island sites, the response to NO concentrations demonstrates the significant effect which the Co(II) and Fe(II) have on the decorated extrinsic semiconductor majority charge carriers as they direct a dominant electron transduction process for reversible electron transduction and chemical sensing (Inverse Hard and Soft acid/base principle) in the absence of significant chemical bond formation. Co(II) and Fe(II) oxide sites enhance response and provide a means for small magnetic fields to interact with and enhance the sensor interface response. For p-type systems, the interaction is with small virtually constant thermal electron populations lying above the Fermi energy at 0 K. The electron removal rate increases with magnetic field strength. At the highest magnetic fields and NO analyte concentrations the available electron population is depleted, and the response to the analyte decreases at higher concentrations. At lower magnetic fields (<1000 G), the response faithfully follows concentration. For n-type systems, the magnetic field interaction increases resistance. This increase in response may be attributed to the interaction with donor levels ∼0.025 eV below the conduction band. A substantial enhancement of sensor response relative to that for the Co(II) and Fe(II) treated PS interfaces is observed, with the introduction of a small magnetic field greatly increasing an already enhanced conductometric response.

  20. Magnetically induced enhancement of reversibly responding conductometric sensors

    NASA Astrophysics Data System (ADS)

    Baker, Caitlin; Laminack, William; Tune, Travis; Gole, James

    2014-04-01

    Small magnetic fields are found to greatly enhance the reversible room temperature conductometric responses of n and p- type porous silicon (PS) interfaces, treated with nanostructured island sites containing paramagnetic Co(II) and Fe(II). At concentrations sufficiently low so as to avoid cross talk between the nanostructured island sites, the response to NO concentrations demonstrates the significant effect which the Co(II) and Fe(II) have on the decorated extrinsic semiconductor majority charge carriers as they direct a dominant electron transduction process for reversible electron transduction and chemical sensing (Inverse Hard and Soft acid/base principle) in the absence of significant chemical bond formation. Co(II) and Fe(II) oxide sites enhance response and provide a means for small magnetic fields to interact with and enhance the sensor interface response. For p-type systems, the interaction is with small virtually constant thermal electron populations lying above the Fermi energy at 0 K. The electron removal rate increases with magnetic field strength. At the highest magnetic fields and NO analyte concentrations the available electron population is depleted, and the response to the analyte decreases at higher concentrations. At lower magnetic fields (<1000 G), the response faithfully follows concentration. For n-type systems, the magnetic field interaction increases resistance. This increase in response may be attributed to the interaction with donor levels ˜0.025 eV below the conduction band. A substantial enhancement of sensor response relative to that for the Co(II) and Fe(II) treated PS interfaces is observed, with the introduction of a small magnetic field greatly increasing an already enhanced conductometric response.

  1. Nonstochastic magnetic reversal in artificial quasicrystalline spin ice

    SciTech Connect

    Farmer, B.; Bhat, V. S.; Woods, J.; Teipel, E.; Smith, N.; De Long, L. E.; Sklenar, J.; Ketterson, J. B.; Hastings, J. T.

    2014-05-07

    We have measured the isothermal DC magnetization of Penrose P2 tilings (P2T) composed of wire segments of permalloy thin film. Micromagnetic simulations reproduce the coercive fields and “knee anomalies” observed in experimental data and show magnetic shape anisotropy constrains segments to be single-domain (Ising spins) at low fields, similar to artificial spin ice (ASI). Mirror symmetry controls the initial reversal of individual segments oriented parallel to the applied field, followed by complex switching of multiple adjacent segments (“avalanches”) of various orientations such that closed magnetization loops (“vortices”) are favored. Ferromagnetic P2T differ from previously studied ASI systems due to their aperiodic translational symmetry and numerous inequivalent pattern vertices, which drive nonstochastic switching of segment polarizations.

  2. Distinguishing magnetic particle size of iron oxide nanoparticles with first-order reversal curves

    SciTech Connect

    Kumari, Monika; Hirt, Ann M.; Widdrat, Marc; Faivre, Damien; Tompa, Éva; Pósfai, Mihály; Uebe, Rene; Schüler, Dirk

    2014-09-28

    Magnetic nanoparticles encompass a wide range of scientific study and technological applications. The success of using the nanoparticles in various applications demands control over size, dispersibility, and magnetics. Hence, the nanoparticles are often characterized by transmission electron microscopy (TEM), X-ray diffraction, and magnetic hysteresis loops. TEM analysis requires a thin layer of dispersed particles on the grid, which may often lead to particle aggregation thus making size analysis difficult. Magnetic hysteresis loops on the other hand provide information on the bulk property of the material without discriminating size, composition, and interaction effects. First order reversal curves (FORCs), described as an assembly of partial hysteresis loops originating from the major loop are efficient in identifying the domain size, composition, and interaction in a magnetic system. This study presents FORC diagrams on a variety of well-characterized biogenic and synthetic magnetite nanoparticles. It also introduces deconvoluted reversible and irreversible components from FORC as an important method for obtaining a semi-quantitative measure of the effective magnetic particle size. This is particularly important in a system with aggregation and interaction among the particles that often leads to either the differences between physical size and effective magnetic size. We also emphasize the extraction of secondary components by masking dominant coercivity fraction on FORC diagram to explore more detailed characterization of nanoparticle systems.

  3. Distinguishing magnetic particle size of iron oxide nanoparticles with first-order reversal curves

    NASA Astrophysics Data System (ADS)

    Kumari, Monika; Widdrat, Marc; Tompa, Éva; Uebe, Rene; Schüler, Dirk; Pósfai, Mihály; Faivre, Damien; Hirt, Ann M.

    2014-09-01

    Magnetic nanoparticles encompass a wide range of scientific study and technological applications. The success of using the nanoparticles in various applications demands control over size, dispersibility, and magnetics. Hence, the nanoparticles are often characterized by transmission electron microscopy (TEM), X-ray diffraction, and magnetic hysteresis loops. TEM analysis requires a thin layer of dispersed particles on the grid, which may often lead to particle aggregation thus making size analysis difficult. Magnetic hysteresis loops on the other hand provide information on the bulk property of the material without discriminating size, composition, and interaction effects. First order reversal curves (FORCs), described as an assembly of partial hysteresis loops originating from the major loop are efficient in identifying the domain size, composition, and interaction in a magnetic system. This study presents FORC diagrams on a variety of well-characterized biogenic and synthetic magnetite nanoparticles. It also introduces deconvoluted reversible and irreversible components from FORC as an important method for obtaining a semi-quantitative measure of the effective magnetic particle size. This is particularly important in a system with aggregation and interaction among the particles that often leads to either the differences between physical size and effective magnetic size. We also emphasize the extraction of secondary components by masking dominant coercivity fraction on FORC diagram to explore more detailed characterization of nanoparticle systems.

  4. Tokamak equilibria with toroidal current reversal: properties and computational issues

    SciTech Connect

    Rodrigues, Paulo; Bizarro, Joao P. S.

    2006-11-30

    Several properties of axisymmetric plasma equilibria with toroidal-current reversal (TCR) are discussed using some unifying concepts from catastrophe theory. Namely, those of structural stability of functions near critical points, singularity unfolding by small perturbations, and model parameter-space division by bifurcation sets are found to be of particular usefulness. Magnetic configurations displaying, simultaneously, TCR and nested flux surfaces are thence shown to be necessarily degenerate and structurally unstable, meaning that they are easily transformed into non-nested ones by small perturbations in the model parameter set. This should lead to a new paradigm when discussing TCR equilibria, as most of present knowledge relies mainly on the properties of nested solutions, which is expected to favor the study of the broader class of non-nested configurations that recently attracted a considerable discussion in the fusion community. In addition, it is also shown how TCR imposes some constraints on plasma profiles, and how these may be dealt with computationally while keeping the ability to manipulate the shape of the inner island system.

  5. Magnetic domain wall gratings for magnetization reversal tuning and confined dynamic mode localization

    NASA Astrophysics Data System (ADS)

    Trützschler, Julia; Sentosun, Kadir; Mozooni, Babak; Mattheis, Roland; McCord, Jeffrey

    2016-08-01

    High density magnetic domain wall gratings are imprinted in ferromagnetic-antiferromagnetic thin films by local ion irradiation by which alternating head-to-tail-to-head-to-tail and head-to-head-to-tail-to-tail spatially overlapping domain wall networks are formed. Unique magnetic domain processes result from the interaction of anchored domain walls. Non-linear magnetization response is introduced by the laterally distributed magnetic anisotropy phases. The locally varying magnetic charge distribution gives rise to localized and guided magnetization spin-wave modes directly constrained by the narrow domain wall cores. The exchange coupled multiphase material structure leads to unprecedented static and locally modified dynamic magnetic material properties.

  6. Magnetic field reversals, polar wander, and core-mantle coupling.

    PubMed

    Courtillot, V; Besse, J

    1987-09-01

    True polar wander, the shifting of the entire mantle relative to the earth's spin axis, has been reanalyzed. Over the last 200 million years, true polar wander has been fast (approximately 5 centimeters per year) most of the time, except for a remarkable standstill from 170 to 110 million years ago. This standstill correlates with a decrease in the reversal frequency of the geomagnetic field and episodes of continental breakup. Conversely, true polar wander is high when reversal frequency increases. It is proposed that intermittent convection modulates the thickness of a thermal boundary layer at the base of the mantle and consequently the core-to-mantle heat flux. Emission of hot thermals from the boundary layer leads to increases in mantle convection and true polar wander. In conjunction, cold thermals released from a boundary layer at the top of the liquid core eventually lead to reversals. Changes in the locations of subduction zones may also affect true polar wander. Exceptional volcanism and mass extinctions at the Cretaceous-Tertiary and Permo-Triassic boundaries may be related to thermals released after two unusually long periods with no magnetic reversals. These environmental catastrophes may therefore be a consequence of thermal and chemical couplings in the earth's multilayer heat engine rather than have an extraterrestrial cause.

  7. Magnetic field reversals, polar wander, and core-mantle coupling.

    PubMed

    Courtillot, V; Besse, J

    1987-09-01

    True polar wander, the shifting of the entire mantle relative to the earth's spin axis, has been reanalyzed. Over the last 200 million years, true polar wander has been fast (approximately 5 centimeters per year) most of the time, except for a remarkable standstill from 170 to 110 million years ago. This standstill correlates with a decrease in the reversal frequency of the geomagnetic field and episodes of continental breakup. Conversely, true polar wander is high when reversal frequency increases. It is proposed that intermittent convection modulates the thickness of a thermal boundary layer at the base of the mantle and consequently the core-to-mantle heat flux. Emission of hot thermals from the boundary layer leads to increases in mantle convection and true polar wander. In conjunction, cold thermals released from a boundary layer at the top of the liquid core eventually lead to reversals. Changes in the locations of subduction zones may also affect true polar wander. Exceptional volcanism and mass extinctions at the Cretaceous-Tertiary and Permo-Triassic boundaries may be related to thermals released after two unusually long periods with no magnetic reversals. These environmental catastrophes may therefore be a consequence of thermal and chemical couplings in the earth's multilayer heat engine rather than have an extraterrestrial cause. PMID:17801638

  8. Magnetic islands at the field reversal surface in reversed field pinches

    SciTech Connect

    Pinsker, R.I.; Reiman, A.H.

    1985-09-01

    In the reversed field pinch (RFP), magnetic field perturbations having zero poloidal mode number and any toroidal mode number are resonant at the field reversal surface. Such perturbations are a particular threat to the RFP because of their weak radial dependence at low toroidal mode number, and because the toroidal field ripple is essentially of this type. The widths of the resulting islands are calculated in this paper. The self-consistent plasma response is included through the assumption that the plasma relaxes to a Taylor force-free state. The connection with linear tearing mode theory is established for those limits where arbitrarily large islands result from infinitesimal perturbations. Toroidal effects are considered, and application of the theory to RFP experiments is discussed.

  9. Magnetic vortex core reversal by excitation of spin waves

    PubMed Central

    Kammerer, Matthias; Weigand, Markus; Curcic, Michael; Noske, Matthias; Sproll, Markus; Vansteenkiste, Arne; Van Waeyenberge, Bartel; Stoll, Hermann; Woltersdorf, Georg; Back, Christian H.; Schuetz, Gisela

    2011-01-01

    Micron-sized magnetic platelets in the flux-closed vortex state are characterized by an in-plane curling magnetization and a nanometer-sized perpendicularly magnetized vortex core. Having the simplest non-trivial configuration, these objects are of general interest to micromagnetics and may offer new routes for spintronics applications. Essential progress in the understanding of nonlinear vortex dynamics was achieved when low-field core toggling by excitation of the gyrotropic eigenmode at sub-GHz frequencies was established. At frequencies more than an order of magnitude higher vortex state structures possess spin wave eigenmodes arising from the magneto-static interaction. Here we demonstrate experimentally that the unidirectional vortex core reversal process also occurs when such azimuthal modes are excited. These results are confirmed by micromagnetic simulations, which clearly show the selection rules for this novel reversal mechanism. Our analysis reveals that for spin-wave excitation the concept of a critical velocity as the switching condition has to be modified. PMID:21505435

  10. Convergence Property of Time Reversal Waves under Noisy Environment

    NASA Astrophysics Data System (ADS)

    Shimura, Takuya; Ochi, Hiroshi

    2004-05-01

    We have studied on the convergence property of time reversal waves (which are equal to phase conjugate waves) in the ocean, particularly in time domain with various configurations of time reversal array (TRA) through simulations and tank experiments. In this paper, the property of time reversal waves under noisy environment is discussed. Simulations were carried out with various sound velocity profiles using the Pekeris solution of the normal mode method and the parabolic equation (PE) method, and tank experiments were also conducted to compare with the simulation results. Results revealed the following. Time reversal waves even at very low signal noise to ratio (SNR) can converge and send the desired signal to the focus at high SNR. The focusing effect of time reversal waves is higher when the horizontal range is extended. If the sound velocity profile is different, the focusing effects are not considerably affected.

  11. Magnetic-field-induced shape recovery by reverse phase transformation.

    PubMed

    Kainuma, R; Imano, Y; Ito, W; Sutou, Y; Morito, H; Okamoto, S; Kitakami, O; Oikawa, K; Fujita, A; Kanomata, T; Ishida, K

    2006-02-23

    Large magnetic-field-induced strains have been observed in Heusler alloys with a body-centred cubic ordered structure and have been explained by the rearrangement of martensite structural variants due to an external magnetic field. These materials have attracted considerable attention as potential magnetic actuator materials. Here we report the magnetic-field-induced shape recovery of a compressively deformed NiCoMnIn alloy. Stresses of over 100 MPa are generated in the material on the application of a magnetic field of 70 kOe; such stress levels are approximately 50 times larger than that generated in a previous ferromagnetic shape-memory alloy. We observed 3 per cent deformation and almost full recovery of the original shape of the alloy. We attribute this deformation behaviour to a reverse transformation from the antiferromagnetic (or paramagnetic) martensitic to the ferromagnetic parent phase at 298 K in the Ni45Co5Mn36.7In13.3 single crystal.

  12. Reversible "triple-Q" elastic field structures in a chiral magnet.

    PubMed

    Hu, Yangfan; Wang, Biao

    2016-01-01

    The analytical solution of the periodic elastic fields in chiral magnets caused by presence of periodically distributed eigenstrains is obtained. For the skyrmion phase, both the periodic displacement field and the stress field are composed of three "triple-Q" structures with different wave numbers. The periodic displacement field, obtained by combining the three "triple-Q" displacement structures, is found to have the same lattice vectors with the magnetic skyrmion lattice. We find that for increasing external magnetic field, one type of "triple-Q" displacement structure and stress structure undergo a "configurational reversal", where the initial and the final field configuration share similar pattern but with opposite direction of all the field vectors. The solution obtained is of fundamental significance for understanding the emergent mechanical properties of skyrmions in chiral magnets. PMID:27457629

  13. Error-field penetration in reversed magnetic shear configurations

    SciTech Connect

    Wang, H. H.; Wang, Z. X.; Wang, X. Q.; Wang, X. G.

    2013-06-15

    Error-field penetration in reversed magnetic shear (RMS) configurations is numerically investigated by using a two-dimensional resistive magnetohydrodynamic model in slab geometry. To explore different dynamic processes in locked modes, three equilibrium states are adopted. Stable, marginal, and unstable current profiles for double tearing modes are designed by varying the current intensity between two resonant surfaces separated by a certain distance. Further, the dynamic characteristics of locked modes in the three RMS states are identified, and the relevant physics mechanisms are elucidated. The scaling behavior of critical perturbation value with initial plasma velocity is numerically obtained, which obeys previously established relevant analytical theory in the viscoresistive regime.

  14. Fabrication of reversibly adhesive fluidic devices using magnetism.

    PubMed

    Rafat, Marjan; Raad, Danielle R; Rowat, Amy C; Auguste, Debra T

    2009-10-21

    Fluidic devices are often made by irreversibly bonding a polydimethylsiloxane (PDMS) mold to itself or a glass substrate by plasma treatment. This method limits the range of materials for fluidic device fabrication and utility for subsequent processing. Here, we present a simple and inexpensive method to fabricate fluidic devices using magnets to reversibly adhere PDMS and other polymer matrices to glass or gel substrates. This approach enables fluidic devices to be fabricated from a variety of materials other than PDMS and glass. Moreover, this method can be used to fabricate composite devices, three-dimensional scaffolds and hydrogel-based fluidic devices.

  15. Suppression/Reversal of Natural Convection by Exploiting the Temperature/Composition Dependence of Magnetic Susceptibility

    NASA Technical Reports Server (NTRS)

    Seybert, C. D.; Evans, J. W.; Leslie, F.; Jones, W. K., Jr.

    2000-01-01

    Natural convection, driven by temperature-or concentration gradients or both, is an inherent phenomenon during solidification of materials on Earth. This convection has practical consequences (e.g effecting macrosegregation) but also renders difficult the scientific examination of diffusive/conductive phenomena during solidification. It is possible to halt, or even reverse, natural convection by exploiting the variation (with temperature, for example) of the susceptibility of a material. If the material is placed in a vertical magnetic field gradient, a buoyancy force of magnetic origin arises and, at a critical field gradient, can balance the normal buoyancy forces to halt convection. At higher field gradients the convection can be reversed. The effect has been demonstrated in experiments at Marshall Space Flight Center where flow was measured by PIV in MnCl2 solution in a superconducting magnet. In auxiliary experiments the field in the magnet and the properties of the solution were measured. Computations of the natural convection, its halting and reversal, using the commercial software FLUENT were in good agreement with the measurements.

  16. Polarity reversals and tilt of the Earth's magnetic dipole

    NASA Technical Reports Server (NTRS)

    Dolginov, A. Z.

    1993-01-01

    There is evidence that the terrestrial magnetic field is connected with the Earth's mantle: (1) there are magnetic anomalies that do not take part in the westward drift of the main field, but are fixed with respect to the mantle; (2) the geomagnetic pole position flips in a particular way by preferred meridional paths during a reversal; and (3) magnetic polarity reversals are correlated with the activations of geological processes. These facts may be explained if we take into account that a significant horizontal temperature gradient can exist in the top levels of the liquid core because of the different thermoconductivity of the different areas of the core-mantle boundary. These temperature inhomogeneities can penetrate the core because fluxes along the core boundary (the thermal wind) can be strongly suppressed by a small redistribution of the chemical composition in the top of the core. The nonparallel gradients of the temperature, density, and composition on the top of the core create a curled electric field that produces a current and a magnetic field. This seed-field can be amplified by motions in the core. The resulting field does not forget the seed-field distribution and in this way the field on the Earth surface (that can be created only in regions with high conductivity, i.e. in the core) is connected with the core-mantle boundary. Contrary to the usual approach to the dynamo problem, we will take into account that the seed field of thermoelectric origin is acting not only at some initial moment of time but permanently.

  17. Recording-media-related morphology and magnetic properties of crystalline CoPt{sub 3} and CoPt{sub 3}-Au core-shell nanoparticles synthesized via reverse microemulsion

    SciTech Connect

    Bahmanrokh, Ghazaleh Hashim, Mansor; Matori, Khamirul Amin; Kanagesan, Samikannu; Sabbaghizadeh, Rahim; Ezzad Shafie, Mohd Shamsul; Navasery, Manizheh; Soltani, Nayereh; Vaziri, Parisa

    2014-09-07

    A comparative experimental study of the magnetic properties of CoPt{sub 3} and CoPt{sub 3}/Au nanoparticles as well as a detailed study of the structural properties of the samples by X-ray diffraction, Transmission electron microscopy, and vibrating sample magnetometer is presented in this work. In addition, the effect of particle size on the structure and magnetic properties of nanoparticles prepared by microemulsion is studied. The correlation between particle size, crystallinity, and magnetization was studied as well. CoPt nanoparticles have been studied intensively over the last decade because of their increased magnetic anisotropy in the ordered phase that can be interesting for high density magnetic recording. A significant high coercivity for as-prepared CoPt{sub 3} and CoPt{sub 3}-Au nanoparticles was obtained at room temperature and enhanced after annealing. The focused aim of our study is to obtain high coercivity at room temperature that follows the Curie-Weiss law. This indicates an interacting system in which the nanoparticles behave like single domain ferromagnetic materials in the particle size range of 8 to 35 nm. In addition, the interaction increases by cooling the samples to low temperature around 15 K. Temperature dependence 1/M graph was obtained to investigate the behavior of nanoparticles at low temperature and shows the best fit with Curie-Weis mode.

  18. Magnetic Reconnection in the MST Reversed Field Pinch

    SciTech Connect

    Crocker, N.E.

    2001-06-01

    Magnetic field line reconnection is a process whereby magnetic field lines which are otherwise topologically preserved by, and frozen into, a plasma can break and reconnect to form field lines with different topologies. It plays a significant role in a wide variety of plasmas, including stellar, space and laboratory plasmas. The focus of this dissertation is the underlying dynamics of reconnection in one particular kind of laboratory plasma: the Reversed Field Pinch (RFP). Specifically, this dissertation reports measurements, made using a pair of insertable diagnostics in conjunction with arrays of magnetic sensing coils positioned near the plasma surface, of the spatial structure of the magnetic and parallel current density fluctuations associated with reconnection in the edge of MST. At least 4 significant results are obtained form such measurements. First we observe direct evidence of reconnection which takes the form of tearing modes in an RFP. Specifically we measure a (radial) magnetic field fluctuation that causes reconnection in the so-called reversal surface, or q = 0 surface, in the edge of MST. Notably this evidence of reconnection at the reversal surface is the first of its kind in an RFP. Second, we measure the radial width of the associated current sheet, or fluctuation in the component of the current density parallel to the equilibrium magnetic field. Such current sheets are a characteristic feature of the reconnection process but their radial widths are sensitive to the specific effects that allow reconnection to occur sometimes call non-ideal effects because reconnection is forbidden by ideal MHD. We compare the observed width to those expected from models of reconnection that incorporate different non-ideal effects in Ohm's law. In particular we see that the observed width is significantly larger than those expected form resistivity in the context of linearly unstable tearing modes and electron inertia. It is a factor of a few larger than the

  19. Local Reversal Durations and Inverse Magnetic Field Patches in Geodynamo Simulations

    NASA Astrophysics Data System (ADS)

    Wicht, J.

    2004-12-01

    Paleomagnetists commonly infer reversal properties based on records from one site only. In an attempt to gain more global information about geomagnetic field reversals Bradford Clement (Nature, 2004) analyses the latitude dependence of reversal durations in several paleomagentic records. He finds that the field transitions takes signifincantly longer close to the poles than near the equator. Such a piece of information is important for testing numerical geodynamo simulations. Many simulated reversals show a comparable latitudinal dependence. These models offer the opportunity to identify the cause of such an effect. I have tried to link the reversal duration to the transitional magnetic field at the core-mantle boundary. Unfortunately, the connection is complex. Reversals tend to last longer then average where the first inverse patches appear at the core-mantel boundary. They are shorter than average where secondary inverse patches tilt over an already weak core-mantel boundary field. Any equatorial and large scale azimuthal transitional field asymmetries can be identified in a global map of reversal duration. It has been speculated that the intensifying inverse patches at the Earth's core-mantel boundary may constitute the start of a field reversal. So far, they are too weak to lead to significant changes in field inclination. This, however, may change if the inverse patches close to the equator move to higher latitudes. Such a behavior is frequently found in dynamo simulations and indeed can mark the start of a field reversal. However, more often the inverse patches disappear again causing only slight oszillations in inclination.

  20. Time resolved transport studies of magnetization reversal in orthogonal spin transfer magnetic tunnel junction devices

    NASA Astrophysics Data System (ADS)

    Wolf, Georg; Chaves-O'Flynn, Gabriel; Kent, Andrew D.; Kardasz, Bartek; Watts, Steve; Pinarbasi, Mustafa

    2014-08-01

    In this work we report on time resolved magnetization reversal driven by spin transfer torque in an orthogonal spin transfer (OST) magnetic tunnel junction device. We focus on the transitions from parallel (P) to antiparallel (AP) states and the reverse transitions (AP to P) under the influence of 10 ns voltage pulses. The electrical response is monitored with a fast real-time oscilloscope and thus timing information of the reversal process is obtained. The P to AP transition switching time decreases with increasing current and shows only direct switching behavior. The AP to P transition shows similar behavior, but has a broader distribution of switching times at high currents. The rare AP to P switching events that occur at later times are due to the occurrence of a pre-oscillation, which could be identified in time resolve voltage traces. A possible origin of these pre-oscillations is seen in micromagnetic simulations, where they are associated with the breakdown of the uniform precession of the magnetization, and lead to reversal of the magnetization at later times.

  1. Inhomogeneities in spin states and magnetization reversal of geometrically identical elongated Co rings

    NASA Astrophysics Data System (ADS)

    Gao, X. S.; Adeyeye, A. O.; Goolaup, S.; Singh, N.; Jung, W.; Castaño, F. J.; Ross, C. A.

    2007-05-01

    The magnetic configurations and magnetic reversal processes in arrays of geometrically identical rounded rectangular Co rings have been investigated. Magnetic imaging reveals a range of configurations, including diagonal onion, horseshoe onion, and vortex states. Reversal from the onion to the vortex state can occur via different routes involving domain wall motion within the rings, and the mechanism depends on the applied field orientation.

  2. Microwave-assisted magnetization reversal using transient precession of magnetization in permalloy hexagons

    NASA Astrophysics Data System (ADS)

    Okano, Genki; Nozaki, Yukio

    2016-06-01

    Microwave-assisted magnetization reversal utilizing a transient precession of magnetization was demonstrated in a permalloy hexagon by applying a 25-ns-wide microwave field and a 500-ps-wide pulsed field with a tunable delay to the microwave field. The switching field in a combination of these two fields becomes smaller than that in only the microwave field, and this additional reduction in switching field oscillates relative to the delay time. From the comparison with the results of micromagnetic simulations, we found that the oscillatory behavior is attributed to the beats in transient precession that occurs in the early stage of microwave-field-induced magnetization excitation.

  3. The magnetic properties of the hollow cylindrical ideal remanence magnet

    NASA Astrophysics Data System (ADS)

    Bjørk, R.

    2016-10-01

    We consider the magnetic properties of the hollow cylindrical ideal remanence magnet. This magnet is the cylindrical permanent magnet that generates a uniform field in the cylinder bore, using the least amount of magnetic energy to do so. The remanence distribution of this magnet is derived and the generated field is compared to that of a Halbach cylinder of equal dimensions. The ideal remanence magnet is shown in most cases to generate a significantly lower field than the equivalent Halbach cylinder, although the field is generated with higher efficiency. The most efficient Halbach cylinder is shown to generate a field exactly twice as large as the equivalent ideal remanence magnet.

  4. Magnetic reversal dynamics of a quantum system on a picosecond timescale

    PubMed Central

    Kuznetsov, Alexey V; Soloviev, Igor I; Bakurskiy, Sergey V; Tikhonova, Olga V

    2015-01-01

    Summary We present our approach for a consistent, fully quantum mechanical description of the magnetization reversal process in natural and artificial atomic systems by means of short magnetic pulses. In terms of the simplest model of a two-level system with a magnetic moment, we analyze the possibility of a fast magnetization reversal on the picosecond timescale induced by oscillating or short unipolar magnetic pulses. We demonstrate the possibility of selective magnetization reversal of a superconducting flux qubit using a single flux quantum-based pulse and suggest a promising, rapid Λ-scheme for resonant implementation of this process. In addition, the magnetization reversal treatment is fulfilled within the framework of the macroscopic theory of the magnetic moment, which allows for the comparison and explanation of the quantum and classical behavior. PMID:26665066

  5. Magnetic reversal dynamics of a quantum system on a picosecond timescale.

    PubMed

    Klenov, Nikolay V; Kuznetsov, Alexey V; Soloviev, Igor I; Bakurskiy, Sergey V; Tikhonova, Olga V

    2015-01-01

    We present our approach for a consistent, fully quantum mechanical description of the magnetization reversal process in natural and artificial atomic systems by means of short magnetic pulses. In terms of the simplest model of a two-level system with a magnetic moment, we analyze the possibility of a fast magnetization reversal on the picosecond timescale induced by oscillating or short unipolar magnetic pulses. We demonstrate the possibility of selective magnetization reversal of a superconducting flux qubit using a single flux quantum-based pulse and suggest a promising, rapid Λ-scheme for resonant implementation of this process. In addition, the magnetization reversal treatment is fulfilled within the framework of the macroscopic theory of the magnetic moment, which allows for the comparison and explanation of the quantum and classical behavior. PMID:26665066

  6. Large reversible magnetocaloric effect in a Ni-Co-Mn-In magnetic shape memory alloy

    NASA Astrophysics Data System (ADS)

    Huang, L.; Cong, D. Y.; Ma, L.; Nie, Z. H.; Wang, Z. L.; Suo, H. L.; Ren, Y.; Wang, Y. D.

    2016-01-01

    Reversibility of the magnetocaloric effect in materials with first-order magnetostructural transformation is of vital significance for practical magnetic refrigeration applications. Here, we report a large reversible magnetocaloric effect in a Ni49.8Co1.2Mn33.5In15.5 magnetic shape memory alloy. A large reversible magnetic entropy change of 14.6 J/(kg K) and a broad operating temperature window of 18 K under 5 T were simultaneously achieved, correlated with the low thermal hysteresis (˜8 K) and large magnetic-field-induced shift of transformation temperatures (4.9 K/T) that lead to a narrow magnetic hysteresis (1.1 T) and small average magnetic hysteresis loss (48.4 J/kg under 5 T) as well. Furthermore, a large reversible effective refrigeration capacity (76.6 J/kg under 5 T) was obtained, as a result of the large reversible magnetic entropy change, broad operating temperature window, and small magnetic hysteresis loss. The large reversible magnetic entropy change and large reversible effective refrigeration capacity are important for improving the magnetocaloric performance, and the small magnetic hysteresis loss is beneficial to reducing energy dissipation during magnetic field cycle in potential applications.

  7. Magnetic domain wall gratings for magnetization reversal tuning and confined dynamic mode localization.

    PubMed

    Trützschler, Julia; Sentosun, Kadir; Mozooni, Babak; Mattheis, Roland; McCord, Jeffrey

    2016-01-01

    High density magnetic domain wall gratings are imprinted in ferromagnetic-antiferromagnetic thin films by local ion irradiation by which alternating head-to-tail-to-head-to-tail and head-to-head-to-tail-to-tail spatially overlapping domain wall networks are formed. Unique magnetic domain processes result from the interaction of anchored domain walls. Non-linear magnetization response is introduced by the laterally distributed magnetic anisotropy phases. The locally varying magnetic charge distribution gives rise to localized and guided magnetization spin-wave modes directly constrained by the narrow domain wall cores. The exchange coupled multiphase material structure leads to unprecedented static and locally modified dynamic magnetic material properties. PMID:27487941

  8. Magnetic domain wall gratings for magnetization reversal tuning and confined dynamic mode localization

    PubMed Central

    Trützschler, Julia; Sentosun, Kadir; Mozooni, Babak; Mattheis, Roland; McCord, Jeffrey

    2016-01-01

    High density magnetic domain wall gratings are imprinted in ferromagnetic-antiferromagnetic thin films by local ion irradiation by which alternating head-to-tail-to-head-to-tail and head-to-head-to-tail-to-tail spatially overlapping domain wall networks are formed. Unique magnetic domain processes result from the interaction of anchored domain walls. Non-linear magnetization response is introduced by the laterally distributed magnetic anisotropy phases. The locally varying magnetic charge distribution gives rise to localized and guided magnetization spin-wave modes directly constrained by the narrow domain wall cores. The exchange coupled multiphase material structure leads to unprecedented static and locally modified dynamic magnetic material properties. PMID:27487941

  9. Influence of the dipolar interactions in the magnetization reversal asymmetry of hard-soft magnetic ribbons

    SciTech Connect

    Rivas, M.; Garcia, J.A.; Tejedor, M.; Bertran, E.; Cespedes, J.G.

    2005-01-15

    Partial crystallization of the metallic glass Co{sub 66}Si{sub 16}B{sub 12}Fe{sub 4}Mo{sub 2} was performed by annealing at temperatures between 500 and 540 deg. C for 10-20 min, resulting in crystallite volume fractions of (0.7-5)x10{sup -3} and sizes of 50-100 nm. This two-phase alloy presents a remarkable feature: a hysteresis loop shift that can be tailored by simply premagnetizing the sample in the adequate magnetic field. Shifts as large as five times the coercive field have been obtained which make them interesting for application as magnetic cores in dc pulse transformers. The asymetrical magnetic reversal is explained in terms of the magnetic dipolar field interaction and the observed hysteresis loops have been satisfactorily simulated by a modification of Stoner-Wohlfarth's model of coherent rotations.

  10. Magnetization reversal studies in structurally tailored cobalt nanowires

    NASA Astrophysics Data System (ADS)

    Kaur, Daljit; Chaudhary, Sujeet; Pandya, Dinesh K.; Gupta, Rekha; Kotnala, R. K.

    2013-10-01

    Cobalt nanowires (NWs) having hcp crystal structure are structurally tailored for different preferred orientations (PO) of (0002), (101¯0), (112¯0) and (101¯1) by varying bath temperature and bath concentration in commercially available 50 nm pore diameter polycarbonate (PCT) and 20 nm pore diameter anodic alumina (AAO) membranes. The magnetization studies show orientation dependent competition of magneto-crystalline anisotropy with shape anisotropy. The large effective anisotropy, Keff (along longitudinal direction) of 1.42×106 erg/cc is observed in (0002) PO NWs, which changes sign (-1.50×106 erg/cc) in (101¯0) PO NWs. The angular dependence of coercivity [HC(θ)] in (0002) oriented Co NWs exhibits a non-monotonic behavior in both the 50 nm and 20 nm samples. The fitting of HC(θ) data reveals that the magnetization reversal mechanism initially takes place by curling and subsequently changes to coherent rotation mode after a certain transition angle, which is higher in case of denser NW array. This increase in transition angle can be attributed to the increased magneto-static interactions in the AAO membrane array having 103 times higher NW areal-density than that in PCT membrane array. Role of dipolar/ magnetostatic anisotropy studied by varying NW areal-density and NW diameter.

  11. Numerical Studies of Magnetization Reversal in Thin Annular Nanorings

    NASA Astrophysics Data System (ADS)

    Chaves-O'Flynn, Gabriel; Kent, Andrew; Stein, Daniel; Bedau, Daniel

    2009-03-01

    The rate of thermally activated magnetization reversal in thin ferromagnetic nanorings has been found analytically in a 1D model in which the demagnetization energy is approximated by a local surface term [1]. Numerical micromagnetic calculations confirm all aspects of the analytic model for narrow thin rings, such as permalloy rings of 200 nm mean radius, 40 nm width and 2 nm thickness [2]. However, the model breaks down in for extremely wide rings, when the ring width approaches its mean diameter. Here we present numerical micromagnetic results for the transition states between the clockwise and counterclockwise state in this limit. We describe how the two transition configurations of narrow rings cease to be saddles of the energy functional. Also, a new low energy metastable state is found to exist for a narrow range of fields. We discuss the results of applying the String Method [3] to determine the transition states and energy barriers between the lowest magnetization configurations of rings. [1] K. Martens, D.L. Stein, and A.D. Kent, PRB 73, 054413 (2006) [2] G. D. Chaves-O'Flynn, D.L. Stein, and A.D. Kent, arXiv:0811.0440 (2008) [3] W. E, W. Ren, E. Vanden-Eijnden, J. Chem. Phys 126, 164103 (2007)

  12. Watermelon-like iron nanoparticles: Cr doping effect on magnetism and magnetization interaction reversal

    SciTech Connect

    Kaur, Maninder; Dai, Qilin; Bowden, Mark E.; Engelhard, Mark H.; Wu, Yaqiao; Tang, Jinke; Qiang, You

    2013-06-26

    Chromium (Cr) forms a solid solution with iron (Fe) lattice when doped in core-shell iron -iron oxide nanocluster (NC) and shows a mixed phase of sigma (σ) FeCr and bcc Fe. The Cr dopant affects heavily the magnetization and magnetic reversal process, and causes the hysteresis loop to shrink near the zero field axis. Dramatic transformation happens from dipolar interaction (0 at. % Cr) to strong exchange interaction (8 at. % of Cr) is confirmed from the Henkel plot and delta M plot, and is explained by a water-melon model of core-shell NC system.

  13. Electrodeposition and magnetic properties of FeCo alloy films

    NASA Astrophysics Data System (ADS)

    Zhou, Dong; Zhou, Mingge; Zhu, Minggang; Yang, Xu; Yue, Ming

    2012-04-01

    FeCo alloys thin films have been successfully electrodeposited on Ag films. The morphology, structure, composition, and magnetic property of the FeCo films were characterized by scanning electron microscopy, x-ray diffraction, induction-coupled plasma spectrometry, vibrating sample magnetometer and network analyzer. The use of reverse pulse current in the process of electrodepostion can reduce the surface roughness obviously. The effects of anodic current density and thickness are studied. The results show that the film fabricated under appropriate conditions has low coercivity and excellent high-frequency magnetic property.

  14. Large Magnetization and Reversible Magnetocaloric Effect at the Second-Order Magnetic Transition in Heusler Materials.

    PubMed

    Singh, Sanjay; Caron, Luana; D'Souza, Sunil Wilfred; Fichtner, Tina; Porcari, Giacomo; Fabbrici, Simone; Shekhar, Chandra; Chadov, Stanislav; Solzi, Massimo; Felser, Claudia

    2016-05-01

    In contrast to rare-earth-based materials, cheaper and more environmentally friendly candidates for cooling applications are found within the family of Ni-Mn Heusler alloys. Initial interest in these materials is focused on the first-order magnetostructural transitions. However, large hysteresis makes a magnetocaloric cycle irreversible. Alternatively, here it is shown how the Heusler family can be used to optimize reversible second-order magnetic phase transitions for magnetocaloric applications. PMID:26928954

  15. Large Magnetization and Reversible Magnetocaloric Effect at the Second-Order Magnetic Transition in Heusler Materials.

    PubMed

    Singh, Sanjay; Caron, Luana; D'Souza, Sunil Wilfred; Fichtner, Tina; Porcari, Giacomo; Fabbrici, Simone; Shekhar, Chandra; Chadov, Stanislav; Solzi, Massimo; Felser, Claudia

    2016-05-01

    In contrast to rare-earth-based materials, cheaper and more environmentally friendly candidates for cooling applications are found within the family of Ni-Mn Heusler alloys. Initial interest in these materials is focused on the first-order magnetostructural transitions. However, large hysteresis makes a magnetocaloric cycle irreversible. Alternatively, here it is shown how the Heusler family can be used to optimize reversible second-order magnetic phase transitions for magnetocaloric applications.

  16. Anomalous magnetization reversal due to proximity effect of antiphase boundaries

    NASA Astrophysics Data System (ADS)

    Sofin, R. G. S.; Wu, Han-Chun; Shvets, I. V.

    2011-12-01

    Here we report anomalous double switching hysteresis loop and high coercivity (˜0.1 T) in Fe3O4(110) thin films. Our analytical model based on spin chains confined within small antiphase boundary domains (APBDs) suggests a significant proximity effect of antiferromagnetic antiphase boundaries (APBs). Furthermore, the calculated domain size (D) follows the well-known scaling relation D=Ct. The results suggest that the interface exchange coupling between neighboring magnetic domains through antiferromagnetic APBs is responsible for the double switching hysteresis. Our findings could help advance the studies of anomalous properties of magnetic materials originating from growth defects. This effect can be utilized for the tunability of exchange bias in devices.

  17. Obtaining Magnetic Properties of Meteorites Using Magnetic Scanner

    NASA Astrophysics Data System (ADS)

    Kletetschka, G.; Nabelek, L.; Mazanec, M.; Simon, K.; Hruba, J.

    2015-12-01

    Magnetic images of Murchison meteorite's and Chelyabinsk meteorite's thin section have been obtained from magnetic scanning system from Youngwood Science and Engineering (YSE) capable of resolving magnetic anomalies down to 10-3 mT range from about 0.3 mm distance between the probe and meteorite surface (resolution about 0.15 mm). Anomalies were produced repeatedly, each time after application of magnetic field pulse of varying amplitude and constant, normal or reversed, direction. This process resulted in both magnetizing and demagnetizing of the meteorite thin section, while keeping the magnetization vector in the plane of the thin section. Analysis of the magnetic data allows determination of coercivity of remanence (Bcr) for the magnetic sources in situ. Value of Bcr is critical for calculating magnetic forces applicable during missions to asteroids where gravity is compromised. Bcr was estimated by two methods. First method measured varying dipole magnetic field strength produced by each anomaly in the direction of magnetic pulses. Second method measured deflections of the dipole direction from the direction of magnetic pulses (Nabelek et al., 2015). Nabelek, L., Mazanec, M., Kdyr, S., and Kletetschka, G., 2015, Magnetic, in situ, mineral characterization of Chelyabinsk meteorite thin section: Meteoritics & Planetary Science.

  18. Modeling Magnetic Properties in EZTB

    NASA Technical Reports Server (NTRS)

    Lee, Seungwon; vonAllmen, Paul

    2007-01-01

    A software module that calculates magnetic properties of a semiconducting material has been written for incorporation into, and execution within, the Easy (Modular) Tight-Binding (EZTB) software infrastructure. [EZTB is designed to model the electronic structures of semiconductor devices ranging from bulk semiconductors, to quantum wells, quantum wires, and quantum dots. EZTB implements an empirical tight-binding mathematical model of the underlying physics.] This module can model the effect of a magnetic field applied along any direction and does not require any adjustment of model parameters. The module has thus far been applied to study the performances of silicon-based quantum computers in the presence of magnetic fields and of miscut angles in quantum wells. The module is expected to assist experimentalists in fabricating a spin qubit in a Si/SiGe quantum dot. This software can be executed in almost any Unix operating system, utilizes parallel computing, can be run as a Web-portal application program. The module has been validated by comparison of its predictions with experimental data available in the literature.

  19. Magnetic interaction reversal in watermelon nanostructured Cr-doped Fe nanoclusters

    SciTech Connect

    Kaur, Maninder; Dai, Qilin; Bowden, Mark; Engelhard, Mark; Wu, Yaqiao; Tang, Jinke; Qiang, You

    2013-01-01

    Cr-doped core-shell Fe/Fe-oxide nanoclusters (NCs) were synthesized at varied atomic percentages of Cr from 0 at. % to 8 at. %. The low concentrations of Cr (<10 at. %) were selected in order to inhibit the complete conversion of the Fe-oxide shell to Cr2O3 and the Fe core to FeCr alloy. The magnetic interaction in Fe/Fe-oxide NCs (rv25 nm) can be controlled by antiferromagnetic Cr-dopant. We report the origin of r-FeCr phase at very low Cr concentration (2 at. %) unlike in previous studies, and the interaction reversal from dipolar to exchange interaction in watermelon-like Cr-doped core-shell NCs. The giant magnetoresistance (GMR) effect,1,2 where an antiferromagnetic (AFM) exchange coupling exists between two ferromagnetic (FM) layers separated by a certain type of magnetic or non-magnetic spacer,3 has significant potential for application in the magnetic recording industry. Soon after the discovery of the GMR, the magnetic properties of multilayer systems (FeCr) became a subject of intensive study. The application of bulk iron-chromium (Fe-Cr) alloys has been of great interest, as these alloys exhibit favorable prop- erties including corrosion resistance, high strength, hardness, low oxidation rate, and strength retention at elevated temper- ature. However, the structural and magnetic properties of Cr-doped Fe nanoclusters (NCs) have not been investigated in-depth. Of all NCs, Fe-based clusters have unique magnetic properties as well as favorable catalytic characteristics in reactivity, selectivity, and durability.4 The incorporation of dopant of varied type and concentration in Fe can modify its chemical ordering, thereby optimizing its electrical, optical, and magnetic properties and opening up many new applications. The substitution of an Fe atom (1.24 A°) by a Cr atom (1.25 A° ) can easily modify the magnetic properties, since (i) the curie temperature (Tc ) of Fe is 1043 K, while Cr is an itinerant AFM with a bulk Neel temperature TN =311 K, and (ii) Fe

  20. Strain-assisted current-induced magnetization reversal in magnetic tunnel junctions: A micromagnetic study with phase-field microelasticity

    SciTech Connect

    Huang, H. B.; Hu, J. M.; Yang, T. N.; Chen, L. Q.; Ma, X. Q.

    2014-09-22

    Effect of substrate misfit strain on current-induced in-plane magnetization reversal in CoFeB-MgO based magnetic tunnel junctions is investigated by combining micromagnetic simulations with phase-field microelasticity theory. It is found that the critical current density for in-plane magnetization reversal decreases dramatically with an increasing substrate strain, since the effective elastic field can drag the magnetization to one of the four in-plane diagonal directions. A potential strain-assisted multilevel bit spin transfer magnetization switching device using substrate misfit strain is also proposed.

  1. Magnetic polarity stratigraphy of the Permian and Carboniferous: The extension of the magnetic reversal record into the Paleozoic

    SciTech Connect

    Opdyke, N.D. )

    1991-03-01

    Magnetic polarity stratigraphy has revolutionized stratigraphic studies in Jurassic to Pleistocene sediments. These studies have been greatly facilitated by the reversal record that is recorded in rocks of the ocean floor. For times prior to the Jurassic, the reversal history of the magnetic field must be determined and eventually related through the type section concept. The magnetic reversal history of the late Paleozoic is dominated by the Permo-Carboniferous reversed superchron (PCRS), which extends from the late Permian to the Carboniferous (Westphalian). Recent studies by the author and his students in Middle Carboniferous sediments of eastern Canada, Pennsylvania, Arizona, and Nevada reveal that the magnetic field has reversed frequently in late Mississippian and early Pennsylvanian times (Meramecian through late Morrowan). The polarity of the magnetic field over this interval is approximately 50% normal and 50% reversed. The frequency of reversal appears to be about one reversal per m.y. The possibility, therefore, exists that this pattern may be used for continental and intercontinental correlation. Attempts are currently underway to correlate this magnetic stratigraphy to fossiliferous marine sections. The base of the PCRS is probably of Atokan age.

  2. Exchange bias effect modified asymmetric magnetization reversal in Ni/YMnO3 multiferroic bilayers

    NASA Astrophysics Data System (ADS)

    Gong, Junlu; Zheng, Dongxing; Li, Dong; Jin, Chao; Li, Peng; Feng, Liefeng; Bai, Haili

    2016-04-01

    Exchange bias (EB) effect modified asymmetric magnetization reversal in Ni/YMnO3 multiferroic bilayers was investigated by combining anisotropic magnetoresistance (AMR) with free energy methods. The promotion and inhibition effects of EB field on magnetization rotation result in the asymmetry of magnetization reversal. The AMR curves exhibit shape transition from arc-like to sin2θH-dependence with increasing external fields due to the competition between Zeeman energy and interfacial coupling energy. The phase shift and asymmetric behaviors become weak as the EB field decreases. Our work suggests that controlling the EB effect can be an alternative way to manipulate the magnetization reversal in exchange biased systems.

  3. Magnetic field reversals in the Milky Way- "cherchez le champ magnetique".

    NASA Astrophysics Data System (ADS)

    Vallee, J. P.

    1996-04-01

    Radio observations of nearby spiral galaxies have tremendously enhanced our knowledge of their global magnetic field distributions. Recent theoretical developments in the area of dynamos have also helped in the interpretation of magnetic field data in spiral galaxies. When it comes to the magnetic field in the Milky Way galaxy, our position in the Milky Way's galactic disk hinders our attempts at interpreting the observational data. This makes the proposition of "cherchez le champ magnetique" a difficult one to follow. Some recent papers have attempted to fit magnetic field models to spiral galaxies, and in particular to the Milky Way galaxy. Magnetic field reversals in the Milky Way are crucial to all interpretations, be they axisymmetric spiral (ASS) or bisymmetric spiral (BSS) global magnetic field models. Magnetic field reversals can be found in both ASS and BSS magnetic field models, not just BSS ones. The axisymmetric spiral (ASS) magnetic field models produced by the dynamo theory already predict magnetic field reversals, and they are of the type observed in the Milky Way. The small number of magnetic field reversals observed in the Milky Way is compatible with the ASS magnetic field models. The bisymmetric spiral (BSS) magnetic field models as applied to the pulsar RM data and to the QSO and galaxies data have many problems, due to the many pitfalls in model fitting the magnetic field reversals observed in the Milky Way. Many pitfalls are discussed here, including the incomplete comparisons of BSS versus ASS models, the number of spiral arms to be used in modelling, and the proper distance to pulsars via the more accurate distribution of thermal electrons within spiral arms. The two magnetic field reversals in our Milky Way are clearly located in the interarm regions. Predicted magnetic field reversals are periodic, while observed ones are not periodic. Magnetic field reversals cannot be masked effectively by local interstellar magnetised shells. The

  4. Space and thickness influence on magnetization reversal in periodic cylinder shaped exchange spring

    NASA Astrophysics Data System (ADS)

    Hu, Chun-lian; Zhou, Yu-cheng; Liao, Leng; Stamps, R. L.

    2015-07-01

    Magnetization reversal in periodic cylinder shaped exchange spring with soft layer Fe3Pt and hard layer FePt has been studied. Coercive field increases with the increase of space between periodic cylinders due to dipole effect in exchange spring Fe3Pt/FePt. Critical field of magnetization reversal decreases with the increase of thickness in soft layer in Fe3Pt/FePt system. This phenomenon is caused by the competition between exchange coupling effect and demagnetization effect. Moreover, from the status of magnetization in different field, magnetization in central region of the periodic cylinders starts to reverse first in periodic cylinder Fe3Pt/FePt exchange spring. The reversion of magnetization from center to boundary is caused by the competition between demagnetization field and magnetic field in periodic cylinder exchange spring.

  5. Robust Magnetic Properties of a Sublimable Single-Molecule Magnet.

    PubMed

    Kiefl, Evan; Mannini, Matteo; Bernot, Kevin; Yi, Xiaohui; Amato, Alex; Leviant, Tom; Magnani, Agnese; Prokscha, Thomas; Suter, Andreas; Sessoli, Roberta; Salman, Zaher

    2016-06-28

    The organization of single-molecule magnets (SMMs) on surfaces via thermal sublimation is a prerequisite for the development of future devices for spintronics exploiting the richness of properties offered by these magnetic molecules. However, a change in the SMM properties due to the interaction with specific surfaces is usually observed. Here we present a rare example of an SMM system that can be thermally sublimated on gold surfaces while maintaining its intact chemical structure and magnetic properties. Muon spin relaxation and ac susceptibility measurements are used to demonstrate that, unlike other SMMs, the magnetic properties of this system in thin films are very similar to those in the bulk, throughout the full volume of the film, including regions near the metal and vacuum interfaces. These results exhibit the robustness of chemical and magnetic properties of this complex and provide important clues for the development of nanostructures based on SMMs. PMID:27139335

  6. Magnetization reversal mechanism of Nd-Fe-B films with perpendicular magnetic anisotropy

    SciTech Connect

    Liu Xiaoxi; Ishida, Go; Morisako, Akimitsu

    2011-04-01

    The microstructure and magnetic properties of Nd-Fe-B films with thicknesses from 100 nm to 3 nm have been investigated. All the films show excellent perpendicular magnetic anisotropy with a squareness ratio of 1 in the perpendicular direction and almost zero coercivity in the in-plane direction. Of particular interest is that the initial magnetization curves sensitively depended on the film thickness. Films thicker than 15 nm show steep initial magnetization curve. Although the films have coercivities larger than 21 kOe, the films can be fully magnetized from the thermally demagnetized state with a field as small as 5 kOe. With the decrease of film thickness to 5 nm, the initial magnetization curve becomes flat. The evolution of initial magnetization curves with film thickness can be understood by the microstructure of the films. Films with thickness of 15 nm show close-packed grains without any intergranular phases. Such microstructures lead to steep initial magnetization curves. On the other hand, when the film thickness decreased to 3 nm, the film thickness became nonuniform. Such microstructure leads to flat initial magnetization curves.

  7. Physical properties of elongated magnetic particles: magnetization and friction coefficient anisotropies.

    PubMed

    Vereda, Fernando; de Vicente, Juan; Hidalgo-Alvarez, Roque

    2009-06-01

    Anisotropy counts: A brief review of the main physical properties of elongated magnetic particles (EMPs) is presented. The most important characteristic of an EMP is the additional contribution of shape anisotropy to the total anisotropy energy of the particle, when compared to spherical magnetic particles. The electron micrograph shows Ni-ferrite microrods fabricated by the authors.We present an overview of the main physical properties of elongated magnetic particles (EMPs), including some of their more relevant properties in suspension. When compared to a spherical magnetic particle, the most important characteristic of an EMP is an additional contribution of shape anisotropy to the total anisotropy energy of the particle. Increasing aspect ratios also lead to an increase in both the critical single-domain size of a magnetic particle and its resistance to thermally activated spontaneous reversal of the magnetization. For single-domain EMPs, magnetization reversal occurs primarily by one of two modes, coherent rotation or curling, the latter being facilitated by larger aspect ratios. When EMPs are used to prepare colloidal suspensions, other physical properties come into play, such as their anisotropic friction coefficient and the consequent enhanced torque they experience in a shear flow, their tendency to align in the direction of an external field, to form less dense sediments and to entangle into more intricate aggregates. From a more practical point of view, EMPs are discussed in connection with two interesting types of magnetic colloids: magnetorheological fluids and suspensions for magnetic hyperthermia. Advances reported in the literature regarding the use of EMPs in these two systems are included. In the final section, we present a summary of the most relevant methods documented in the literature for the fabrication of EMPs, together with a list of the most common ferromagnetic materials that have been synthesized in the form of EMPs. PMID:19434654

  8. Physical properties of elongated magnetic particles: magnetization and friction coefficient anisotropies.

    PubMed

    Vereda, Fernando; de Vicente, Juan; Hidalgo-Alvarez, Roque

    2009-06-01

    Anisotropy counts: A brief review of the main physical properties of elongated magnetic particles (EMPs) is presented. The most important characteristic of an EMP is the additional contribution of shape anisotropy to the total anisotropy energy of the particle, when compared to spherical magnetic particles. The electron micrograph shows Ni-ferrite microrods fabricated by the authors.We present an overview of the main physical properties of elongated magnetic particles (EMPs), including some of their more relevant properties in suspension. When compared to a spherical magnetic particle, the most important characteristic of an EMP is an additional contribution of shape anisotropy to the total anisotropy energy of the particle. Increasing aspect ratios also lead to an increase in both the critical single-domain size of a magnetic particle and its resistance to thermally activated spontaneous reversal of the magnetization. For single-domain EMPs, magnetization reversal occurs primarily by one of two modes, coherent rotation or curling, the latter being facilitated by larger aspect ratios. When EMPs are used to prepare colloidal suspensions, other physical properties come into play, such as their anisotropic friction coefficient and the consequent enhanced torque they experience in a shear flow, their tendency to align in the direction of an external field, to form less dense sediments and to entangle into more intricate aggregates. From a more practical point of view, EMPs are discussed in connection with two interesting types of magnetic colloids: magnetorheological fluids and suspensions for magnetic hyperthermia. Advances reported in the literature regarding the use of EMPs in these two systems are included. In the final section, we present a summary of the most relevant methods documented in the literature for the fabrication of EMPs, together with a list of the most common ferromagnetic materials that have been synthesized in the form of EMPs.

  9. Reverse osmosis membrane of high urea rejection properties. [water purification

    NASA Technical Reports Server (NTRS)

    Johnson, C. C.; Wydeven, T. J. (Inventor)

    1980-01-01

    Polymeric membranes suitable for use in reverse osmosis water purification because of their high urea and salt rejection properties are prepared by generating a plasma of an unsaturated hydrocarbon monomer and nitrogen gas from an electrical source. A polymeric membrane is formed by depositing a polymer of the unsaturated monomer from the plasma onto a substrate, so that nitrogen from the nitrogen gas is incorporated within the polymer in a chemically combined form.

  10. Magnetic phase transitions and magnetization reversal in MnRuP

    NASA Astrophysics Data System (ADS)

    Lampen-Kelley, P.; Mandrus, D.

    The ternary phosphide MnRuP is an incommensurate antiferromagnetic metal crystallizing in the non-centrosymmetric Fe2P-type crystal structure. Below the Neel transition at 250 K, MnRuP exhibits hysteretic anomalies in resistivity and magnetic susceptibility curves as the propagation vectors of the spiral spin structure change discontinuously across T1 = 180 K and T2 = 100 K. Temperature-dependent X-ray diffraction data indicate that the first-order spin reorientation occurs in the absence of a structural transition. A strong magnetization reversal (MR) effect is observed upon cooling the system through TN in moderate dc magnetic fields. Positive magnetization is recovered on further cooling through T1 and maintained in subsequent warming curves. The field dependence and training of the MR effect in MnRuP will be discussed in terms of the underlying magnetic structures and compared to anomalous MR observed in vanadate systems. This work is supported by the Gordon and Betty Moore Foundation GBMF4416 and U.S. DOE, Office of Science, BES, Materials Science and Engineering Division.

  11. Magnetic domain structure and magnetization reversal in submicron-scale Co dots

    SciTech Connect

    Fernandez, A., LLNL

    1998-02-17

    We present a magnetic force microscopy (MFM) analysis of arrays of submicron-scale Co dots fabricated by interference lithography. The dots are thin (180-300 A) and are elliptical in shape. MFM of these structures reveals that they relax into highly ordered remanent states whose symmetry and configuration are governed by their shape anisotropy. In particular, when the dots are saturated along the easy-axis, a uniformly magnetized state persists at remanence. However, when the dots are saturated in hard-axis, they relax into a single-vortex state in which the circulation can have either sign. Both remanent states are characterized by smoothly varying magnetization patterns and a high degree of uniformity across the array. We attribute the ordered behavior of these structures to the film microstructure, which allows the shape anisotropy to dominate over magnetocrystalline anisotropy. By imaging a series of minor-loop remanent states, we show that magnetization reversal in these structures occurs via the nucleation and annihilation of a single vortex. Magnetic hysteresis loop measurements are consistent with these observations and provide additional details. Furthermore, we present the results of micromagnetic simulations, which are in excellent agreement with both the MFM images and the hysteresis loop measurements.

  12. Magnetic domain structure and magnetization reversal in submicron-scale Co dots

    SciTech Connect

    Cerjan, C J; Fernandez, A; Gibbons, M; Wall, M A

    1998-09-24

    We present a magnetic force microscopy (MFM) analysis of arrays of submicron-scale Co dots fabricated by interference lithography. The dots are thin (180--300 Å) and elliptical in shape. MFM reveals that these structures relax into highly ordered remanent states whose symmetry and configuration are governed by their shape anisotropy. In particular, when the dots are saturated along their long-axis, a uniformly magnetized state persists at remanence. However, when the dots are saturated along their short-axis, they relax into a single-vortex state in which the circulation can have either sign. Both states are characterized by smoothly varying magnetization patterns and a high degree of uniformity across the array. We attribute the ordered behavior of these.structures to the film microstructure, which allows the shape anisotropy to dominate over magnetocrystalline anjsotropy. By imaging a series of minor-loop remanent states, we show that magnetization reversal in these structures occurs via the nucleation and annihilation of a single vortex. Magnetic hysteresis loop measurements are consistent with these observations and provide additional details. Furthermore, we present the results of micromagnetic simulations, which are in excellent agreement with both the MFM images and the hysteresis loop measurements. © 1998 Elsevier Science B.V. All rights reserved.

  13. A detailed study of magnetization reversal in individual Ni nanowires

    SciTech Connect

    Vilanova Vidal, Enrique; Ivanov, Yurii P.; Mohammed, Hanan; Kosel, Jürgen

    2015-01-19

    Magnetic nanowires have emerged as essential components for a broad range of applications. In many cases, a key property of these components is the switching field, which is studied as a function of the angle between the field and the nanowire. We found remarkable differences of up to 100% between the switching fields of different nanowires from the same fabrication batch. Our experimental results and micromagnetic simulations indicate that the nanowires exhibit a single domain behavior and that the switching mechanism includes vortex domain wall motion across the nanowire. The differences between the switching fields are attributed to different cross-sections of the nanowires, as found by electron microscopy. While a circular cross-section yields the smallest switching field values, any deviation from this shape results in an increase of the switching field. The shape of the nanowires' cross-sections is thus a critical parameter that has not been previously taken into account.

  14. Nanoscale imaging of magnetization reversal driven by spin-orbit torque

    NASA Astrophysics Data System (ADS)

    Gilbert, Ian; Chen, P. J.; Gopman, Daniel B.; Balk, Andrew L.; Pierce, Daniel T.; Stiles, Mark D.; Unguris, John

    2016-09-01

    We use scanning electron microscopy with polarization analysis to image deterministic, spin-orbit torque-driven magnetization reversal of in-plane magnetized CoFeB rectangles in zero applied magnetic field. The spin-orbit torque is generated by running a current through heavy metal microstrips, either Pt or Ta, upon which the CoFeB rectangles are deposited. We image the CoFeB magnetization before and after a current pulse to see the effect of spin-orbit torque on the magnetic nanostructure. The observed changes in magnetic structure can be complex, deviating significantly from a simple macrospin approximation, especially in larger elements. Overall, however, the directions of the magnetization reversal in the Pt and Ta devices are opposite, consistent with the opposite signs of the spin Hall angles of these materials. Our results elucidate the effects of current density, geometry, and magnetic domain structure on magnetization switching driven by spin-orbit torque.

  15. Time-resolved imaging of pulse-induced magnetization reversal with a microwave assist field

    PubMed Central

    Rao, Siddharth; Rhensius, Jan; Bisig, Andre; Mawass, Mohamad-Assaad; Weigand, Markus; Kläui, Mathias; Bhatia, Charanjit S.; Yang, Hyunsoo

    2015-01-01

    The reversal of the magnetization under the influence of a field pulse has been previously predicted to be an incoherent process with several competing phenomena such as domain wall relaxation, spin wave-mediated instability regions, and vortex-core mediated reversal dynamics. However, there has been no study on the direct observation of the switching process with the aid of a microwave signal input. We report a time-resolved imaging study of magnetization reversal in patterned magnetic structures under the influence of a field pulse with microwave assistance. The microwave frequency is varied to demonstrate the effect of resonant microwave-assisted switching. We observe that the switching process is dominated by spin wave dynamics generated as a result of magnetic instabilities in the structures, and identify the frequencies that are most dominant in magnetization reversal. PMID:26023723

  16. Electric-field-driven magnetization reversal in square-shaped nanomagnet-based multiferroic heterostructure

    SciTech Connect

    Peng, Ren-Ci; Nan, Ce-Wen E-mail: cwnan@tsinghua.edu.cn; Wang, J. J. E-mail: cwnan@tsinghua.edu.cn; Chen, Long-Qing; Hu, Jia-Mian

    2015-04-06

    Based on phase field modeling and thermodynamic analysis, purely electric-field-driven magnetization reversal was shown to be possible in a multiferroic heterostructure of a square-shaped amorphous Co{sub 40}Fe{sub 40}B{sub 20} nanomagnet on top of a ferroelectric layer through electrostrain. The reversal is made possible by engineering the mutual interactions among the built-in uniaxial magnetic anisotropy, the geometry-dependent magnetic configuration anisotropy, and the magnetoelastic anisotropy. Particularly, the incorporation of the built-in uniaxial anisotropy made it possible to reverse magnetization with one single unipolar electrostrain pulse, which is simpler than previous designs involving the use of bipolar electrostrains and may alleviate ferroelectric fatigue. Critical conditions for triggering the magnetization reversal are identified.

  17. Magnetic and electrical properties of Martian particles

    NASA Technical Reports Server (NTRS)

    Olhoeft, G. R.

    1991-01-01

    The only determinations of the magnetic properties of Martian materials come from experiments on the two Viking Landers. The results suggest Martian soil containing 1 to 10 percent of a highly magnetic phase. Though the magnetic phase mineral was not conclusively identified, the predominate interpretation is that the magnetic phase is probably maghemite. The electrical properties of the surface of Mars were only measured remotely by observations with Earth based radar, microwave radiometry, and inference from radio-occultation of Mars orbiting spacecraft. No direct measurements of electrical properties on Martian materials have been performed.

  18. Influence of internal geometry on magnetization reversal in asymmetric permalloy rings

    NASA Astrophysics Data System (ADS)

    Gopman, D. B.; Kabanov, Y. P.; Cui, J.; Lynch, C. S.; Shull, R. D.

    2016-08-01

    We report the magnetization reversal behavior of microstructured Ni80Fe20 rings using magneto-optic indicator film imaging and magnetometry. While the reversal behavior of rings with a symmetric (circular) interior hole agrees with micromagnetic simulations of an onion → vortex → onion transition, we experimentally demonstrate that rings possessing an elliptical hole with an aspect ratio of 2 exhibit complex reversal behavior comprising incoherent domain propagation in the rings. Magneto optic images reveal metastable magnetic configurations that illustrate this incoherent behavior. These results have important implications for understanding the reversal behavior of asymmetric ferromagnetic rings.

  19. Optical Writing of Magnetic Properties by Remanent Photostriction.

    PubMed

    Iurchuk, V; Schick, D; Bran, J; Colson, D; Forget, A; Halley, D; Koc, A; Reinhardt, M; Kwamen, C; Morley, N A; Bargheer, M; Viret, M; Gumeniuk, R; Schmerber, G; Doudin, B; Kundys, B

    2016-09-01

    We present an optically induced remanent photostriction in BiFeO_{3}, resulting from the photovoltaic effect, which is used to modify the ferromagnetism of Ni film in a hybrid BiFeO_{3}/Ni structure. The 75% change in coercivity in the Ni film is achieved via optical and nonvolatile control. This photoferromagnetic effect can be reversed by static or ac electric depolarization of BiFeO_{3}. Hence, the strain dependent changes in magnetic properties are written optically, and erased electrically. Light-mediated straintronics is therefore a possible approach for low-power multistate control of magnetic elements relevant for memory and spintronic applications.

  20. Optical Writing of Magnetic Properties by Remanent Photostriction

    NASA Astrophysics Data System (ADS)

    Iurchuk, V.; Schick, D.; Bran, J.; Colson, D.; Forget, A.; Halley, D.; Koc, A.; Reinhardt, M.; Kwamen, C.; Morley, N. A.; Bargheer, M.; Viret, M.; Gumeniuk, R.; Schmerber, G.; Doudin, B.; Kundys, B.

    2016-09-01

    We present an optically induced remanent photostriction in BiFeO3 , resulting from the photovoltaic effect, which is used to modify the ferromagnetism of Ni film in a hybrid BiFeO3/Ni structure. The 75% change in coercivity in the Ni film is achieved via optical and nonvolatile control. This photoferromagnetic effect can be reversed by static or ac electric depolarization of BiFeO3 . Hence, the strain dependent changes in magnetic properties are written optically, and erased electrically. Light-mediated straintronics is therefore a possible approach for low-power multistate control of magnetic elements relevant for memory and spintronic applications.

  1. Optical Writing of Magnetic Properties by Remanent Photostriction.

    PubMed

    Iurchuk, V; Schick, D; Bran, J; Colson, D; Forget, A; Halley, D; Koc, A; Reinhardt, M; Kwamen, C; Morley, N A; Bargheer, M; Viret, M; Gumeniuk, R; Schmerber, G; Doudin, B; Kundys, B

    2016-09-01

    We present an optically induced remanent photostriction in BiFeO_{3}, resulting from the photovoltaic effect, which is used to modify the ferromagnetism of Ni film in a hybrid BiFeO_{3}/Ni structure. The 75% change in coercivity in the Ni film is achieved via optical and nonvolatile control. This photoferromagnetic effect can be reversed by static or ac electric depolarization of BiFeO_{3}. Hence, the strain dependent changes in magnetic properties are written optically, and erased electrically. Light-mediated straintronics is therefore a possible approach for low-power multistate control of magnetic elements relevant for memory and spintronic applications. PMID:27636494

  2. Resonance and Chaotic Trajectories in Magnetic Field Reversed Configuration

    SciTech Connect

    A.S. Landsman; S.A. Cohen; M. Edelman; G.M. Zaslavsky

    2005-04-13

    The nonlinear dynamics of a single ion in a field-reversed configuration (FRC) were investigated. FRC is a toroidal fusion device which uses a specific type of magnetic field to confine ions. As a result of angular invariance, the full three-dimensional Hamiltonian system can be expressed as two coupled, highly nonlinear oscillators. Due to the high nonlinearity in the equations of motion, the behavior of the system is extremely complex, showing different regimes, depending on the values of the conserved canonical angular momentum and the geometry of the fusion vessel. Perturbation theory and averaging were used to derive the unperturbed Hamiltonian and frequencies of the two degrees of freedom. The derived equations were then used to find resonances and compare to Poincar{copyright} surface-of-section plots. A regime was found where the nonlinear resonances were clearly separated by KAM [Kolmogorov-Arnold-Mosher] curves. The structure of the observed island chains was explained. The condition for the destruction of KAM curves and the onset of strong chaos was derived, using Chirikov island overlap criterion, and shown qualitatively to depend both on the canonical angular momentum and geometry of the device. After a brief discussion of the adiabatic regime the paper goes on to explore the degenerate regime that sets in at higher values of angular momenta. In this regime, the unperturbed Hamiltonian can be approximated as two uncoupled linear oscillators. In this case, the system is near-integrable, except in cases of a universal resonance, which results in large island structures, due to the smallness of nonlinear terms, which bound the resonance. The linear force constants, dominant in this regime, were derived and the geometry for a large one-to-one resonance identified. The above analysis showed good agreement with numerical simulations and was able to explain characteristic features of the dynamics.

  3. Emergent properties of magnetic materials

    NASA Astrophysics Data System (ADS)

    Ratcliff, William Davis, II

    In Tolstoy's War and Peace, history is presented as a tapestry spun from the daily interactions of large numbers of individuals. Even if one understands individuals, it is very difficult to predict history. Similarly, the interactions of large numbers of electrons give rise to properties that one would not initially guess from their microscopic interactions. During the course of my dissertation, I have explored emergent phenomena in a number of contexts. In ZnCr2O4, geometric frustration gives rise to a plethora of equivalent ground states. From these, a lower dimensional set of collinear spins on hexagons are selected to form the building blocks of the lattice. In MgTi2O4, quantum spins dimerize and form a unique chiral ordering pattern on the spinel lattice. Descending into two dimensions, differences in size and charge give rise to an ordering between triangular layers of magnetic and nonmagnetic ions. This triangular lattice allows for the possibility of observing the RVB spin liquid state, or perhaps a valence bond crystal and initial measurements are promising. Also, on the spinel lattice, ionic ordering gives rise to one dimensional chains with their own interesting physics. Finally, in the SrCoxTi1-x O3, system we find that upon reduction, tiny clusters of Co metal precipitate out and chemical inhomogeneity on the microscale may determine much of the physics. This has relevance to a number of recent claims of room temperature ferromagnism in dilute magnetic systems. In all of these systems, complex behavior emerges from well understood microscopic behavior. For me, this is the fascination of strongly correlated electronic systems.

  4. Soft and hard natures of Nd2Fe14B permanent magnet explored by first-order-reversal-curves

    NASA Astrophysics Data System (ADS)

    Chen, Po-An; Yang, Chao-Yao; Chang, Shu-Jui; Lee, Min-Han; Tang, Nai-Kuang; Yen, Sheng-Chan; Tseng, Yuan-Chieh

    2014-12-01

    Two commercial Nd2Fe14B samples, MQP-B and sintered-NdFeB were investigated using synchrotron-based x-ray diffraction and first-order-reversal-curves (FORCs). Despite differing in magnetic and structural properties, the two samples were found to comprise two major ferromagnetic components in FORCs. For the sintered-NdFeB case, the soft component may originate from the intrinsically soft Nd-f site which was coupled with its local Fe atomic environment that differs in magnetic anisotropy from the Nd-g site (intrinsically hard). It may directly originate from the Nd-rich phase or microstructural imperfection, while the former possibility (Nd-f site) appears greater than the latter. While for the MQP-B, the minor second phase resulting from high structural disorder was likely in charge of the presence of the soft component. Sophisticated FORCs analyses revealed the natures of the soft and hard components, soft-hard coupling and switching reversibility of the two cases, irrespective of the origins of their two components. This provides insights to the origin of magnetic stability and reversal dynamics of Nd2Fe14B that have not been fully understood by conventional magnetic analyses. The coexistence of the two components led to an incoherent reversal undermining the magnetic stability of Nd2Fe14B. This is a fundamental problem as to why the performance extremity can only be improved finitely through extrinsic tuning. From FORCs simulation we understand that the soft-hard coupling was moderate in a real Nd2Fe14B compound. A stronger soft-hard coupling is necessary to conquer the anisotropic competition to enable a coherent reversal that will promote the magnetic hardness.

  5. Simulating magnetic nanotubes using a chain of ellipsoid-rings model with a magnetization reversal process by fanning rotation.

    PubMed

    Wang, Jieqiong; Yang, Sen; Gong, Junfeng; Xu, Minwei; Adil, Murtaza; Wang, Yu; Zhang, Yin; Song, Xiaoping; Zeng, Hao

    2015-04-21

    Recently, magnetic nanotubes have attracted great attention owing to the advantages of tubular geometry. Of all the physical properties of magnetic nanotubes, the magnetic behavior plays a pivotal role in potential applications, particularly in biotechnology. Modeling magnetic nanotubes provides an effective way to determine the geometry dependent magnetic properties. In the present article, we model the nanotube as a chain of ellipsoid-rings; thus the magnetic behavior of nanotubes is simulated by the fanning rotation of magnetic moments. Based on this model, we further discuss the influence of tubular geometric parameters on the magnetic properties. The calculated magnetic properties of Fe, Co, Ni, Fe3O4 and CoFe2O4 nanotubes are all consistent with their experimental data. Consequently, our model provides an easy and general approach to magnetic nanotubes.

  6. Aspect-ratio dependence of magnetization reversal in cylindrical ferromagnetic nanowires

    NASA Astrophysics Data System (ADS)

    Sultan, Musaab S.; Atkinson, Del

    2016-05-01

    The magnetization reversal behavior in isolated cylindrical and square cross-section Ni81Fe19 nanowires was systematically studied as a function of nanowire cross-section dimensions from 10 up to 200 nm using micromagnetic simulations. This approach provides access to the switching field, remanence ratio and most significantly the magnetization structures during reversal, which allows the evolution of magnetization processes to be studied with scaling of the cross-sectional dimensions. The dimensional trends in reversal behavior for both square and circular cross-section were comparable throughout the range of dimensions studied. The thinnest nanowires showed simple square switching and 100% remanence. With increasing diameter the switching field reduces and above 40 nm the reversal behavior shows an increasing rotational component prior to sharp switching of the magnetization. The magnitude of the reversible component increases with increasing dimensions up to 150 nm, above which the magnetization reversal process is more complicated and the hysteresis loops are no longer bistable. The micromagnetic structures evolve from simple uniform parallel single domain states in the thinnest wires through the formation of vortex-like end states in thicker wires to complex multidomain structures during the reversal of the thickest wires. In the later cases the reversal is not simple curling-like behavior, although the angular switching field dependence was comparable with curling.

  7. Magnetization reversal assisted by half antivortex states in nanostructured circular cobalt disks

    SciTech Connect

    Lara, A.; Aliev, F. G.; Dobrovolskiy, O. V.; Prieto, J. L.; Huth, M.

    2014-11-03

    The half antivortex, a fundamental topological structure which determines magnetization reversal of submicron magnetic devices with domain walls, has been suggested also to play a crucial role in spin torque induced vortex core reversal in circular disks. Here, we report on magnetization reversal in circular disks with nanoholes through consecutive metastable states with half antivortices. In-plane anisotropic magnetoresistance and broadband susceptibility measurements accompanied by micromagnetic simulations reveal that cobalt (Co) disks with two and three linearly arranged nanoholes directed at 45° and 135° with respect to the external magnetic field show reproducible step-like changes in the anisotropic magnetoresistance and magnetic permeability due to transitions between different intermediate states mediated by vortices and half antivortices confined to the dot nanoholes and edges, respectively. Our findings are relevant for the development of multi-hole based spintronic and magnetic memory devices.

  8. Magnetic Reversal of Electric Polarization with Fixed Chirality of Magnetic Structure in a Chiral-Lattice Helimagnet MnSb_{2}O_{6}.

    PubMed

    Kinoshita, M; Seki, S; Sato, T J; Nambu, Y; Hong, T; Matsuda, M; Cao, H B; Ishiwata, S; Tokura, Y

    2016-07-22

    The correlation between magnetic and dielectric properties has been investigated for the single crystal of the chiral triangular-lattice helimagnet MnSb_{2}O_{6}. We found that the spin-spiral plane in the ground state has a considerable tilting from the (110) plane and that the sign of the spin-spiral tilting angle is coupled to the clockwise or counterclockwise manner of spin rotation and accordingly to the sign of magnetically induced electric polarization. This leads to unique magnetoelectric responses such as the magnetic-field-induced selection of a single ferroelectric domain as well as the reversal of electric polarization just by a slight tilting of the magnetic field direction, where the chiral nature of the crystal structure plays a crucial role through the coupling of the chirality between the crystal and magnetic structures. Our results demonstrate that crystallographic chirality can be an abundant source of novel magnetoelectric functions with coupled internal degrees of freedom. PMID:27494497

  9. Magnetic Reversal of Electric Polarization with Fixed Chirality of Magnetic Structure in a Chiral-Lattice Helimagnet MnSb2 O6

    NASA Astrophysics Data System (ADS)

    Kinoshita, M.; Seki, S.; Sato, T. J.; Nambu, Y.; Hong, T.; Matsuda, M.; Cao, H. B.; Ishiwata, S.; Tokura, Y.

    2016-07-01

    The correlation between magnetic and dielectric properties has been investigated for the single crystal of the chiral triangular-lattice helimagnet MnSb2 O6 . We found that the spin-spiral plane in the ground state has a considerable tilting from the (110) plane and that the sign of the spin-spiral tilting angle is coupled to the clockwise or counterclockwise manner of spin rotation and accordingly to the sign of magnetically induced electric polarization. This leads to unique magnetoelectric responses such as the magnetic-field-induced selection of a single ferroelectric domain as well as the reversal of electric polarization just by a slight tilting of the magnetic field direction, where the chiral nature of the crystal structure plays a crucial role through the coupling of the chirality between the crystal and magnetic structures. Our results demonstrate that crystallographic chirality can be an abundant source of novel magnetoelectric functions with coupled internal degrees of freedom.

  10. High temperature structural and magnetic properties of cobalt nanorods

    SciTech Connect

    Ait Atmane, Kahina; Zighem, Fatih; Soumare, Yaghoub; Ibrahim, Mona; Boubekri, Rym; Maurer, Thomas; Margueritat, Jeremie; Piquemal, Jean-Yves; Ott, Frederic; Chaboussant, Gregory; Schoenstein, Frederic; Jouini, Noureddine; Viau, Guillaume

    2013-01-15

    We present in this paper the structural and magnetic properties of high aspect ratio Co nanoparticles ({approx}10) at high temperatures (up to 623 K) using in-situ X ray diffraction (XRD) and SQUID characterizations. We show that the anisotropic shapes, the structural and texture properties are preserved up to 500 K. The coercivity can be modelled by {mu}{sub 0}H{sub C}=2(K{sub MC}+K{sub shape})/M{sub S} with K{sub MC} the magnetocrystalline anisotropy constant, K{sub shape} the shape anisotropy constant and M{sub S} the saturation magnetization. H{sub C} decreases linearly when the temperature is increased due to the loss of the Co magnetocrystalline anisotropy contribution. At 500 K, 50% of the room temperature coercivity is preserved corresponding to the shape anisotropy contribution only. We show that the coercivity drop is reversible in the range 300-500 K in good agreement with the absence of particle alteration. Above 525 K, the magnetic properties are irreversibly altered either by sintering or by oxidation. - Graphical abstract: We present in this paper the structural and magnetic properties of high aspect ratio Co nanorods ({approx}10) at high temperatures (up to 623 K) using in-situ X-ray diffraction and SQUID characterizations. We show that the anisotropic shapes, the structural and texture properties are preserved up to 500 K. Above 525 K, the magnetic properties are irreversibly altered either by sintering or by oxidation. Highlights: Black-Right-Pointing-Pointer Ferromagnetic Co nanorods are prepared using the polyol process. Black-Right-Pointing-Pointer The structural and texture properties of the Co nanorods are preserved up to 500 K. Black-Right-Pointing-Pointer The magnetic properties of the Co nanorods are irreversibly altered above 525 K.

  11. Onset of a propagating self-sustained spin reversal front in a magnetic system.

    PubMed

    Subedi, P; Vélez, S; Macià, F; Li, S; Sarachik, M P; Tejada, J; Mukherjee, S; Christou, G; Kent, A D

    2013-05-17

    The energy released in a magnetic material by reversing spins as they relax toward equilibrium can lead to a dynamical instability that ignites self-sustained rapid relaxation along a deflagration front that propagates at a constant subsonic speed. Using a trigger heat pulse and transverse and longitudinal magnetic fields, we investigate and control the crossover between thermally driven magnetic relaxation and magnetic deflagration in single crystals of Mn(12)-acetate. PMID:25167444

  12. Onset of a propagating self-sustained spin reversal front in a magnetic system.

    PubMed

    Subedi, P; Vélez, S; Macià, F; Li, S; Sarachik, M P; Tejada, J; Mukherjee, S; Christou, G; Kent, A D

    2013-05-17

    The energy released in a magnetic material by reversing spins as they relax toward equilibrium can lead to a dynamical instability that ignites self-sustained rapid relaxation along a deflagration front that propagates at a constant subsonic speed. Using a trigger heat pulse and transverse and longitudinal magnetic fields, we investigate and control the crossover between thermally driven magnetic relaxation and magnetic deflagration in single crystals of Mn(12)-acetate.

  13. Magnetization Reversal Process of Single Crystal α-Fe Containing a Nonmagnetic Particle

    SciTech Connect

    Li, Yi; Xu, Ben; Hu, Shenyang Y.; Li, Yulan; Li, Qiu-Lin; Liu, Wei

    2015-09-25

    The magnetization reversal process and hysteresis loops in a single crystal α-iron with nonmagnetic particles are simulated in this work based on the Landau-Lifshitz–Gilbert equation. The evolutions of the magnetic domain morphology are studied, and our analyses show that the magnetization reversal process is affected by the interaction between the moving domain wall and the existing nonmagnetic particles. This interaction strongly depends on the size of the particles, and it is found that particles with a particular size contribute the most to magnetic hardening.

  14. In Situ Transmission Electron Microscopy Studies of the Magnetization Reversal Mechanism in Information Storage Materials.

    PubMed

    Petford-Long; Portier; Bayle-Guillemaud; Anthony; Brug

    1998-05-01

    : The Foucault and Fresnel modes of Lorentz microscopy, together with a quantitative magnetization mapping technique, summed image differential phase-contrast imaging, were used to study the magnetization reversal mechanism of the sense layer in spin-valve structures exhibiting the giant magnetoresistance effect. In addition to studies of sheet film, lithographically defined spin-valve elements were investigated. A current can be passed through the element during magnetizing so that the effect of the applied current on the giant magnetoresistance and magnetization reversal mechanism can be studied. Results are presented for a number of different spin-valve structures. PMID:9767670

  15. Polarity reversal of a magnetic vortex core by a unipolar, non-resonant in-plane pulsed magnetic field.

    SciTech Connect

    Keavney, D. J.; Cheng, X. M.; Buchanan, K. S.

    2009-06-24

    We report the polarity reversal of a magnetic vortex core using a nonresonant in-plane pulsed magnetic field of arbitrary waveform studied using time-resolved x-ray photoemission electron microscopy and micromagnetic simulations. The imaging and simulations show that a 5 mT pulse, higher than the critical field for nonlinear effects, effectively leads to the randomization of the vortex core polarity. The micromagnetic simulations further show that the onset of stochastic core polarity randomization does not necessarily coincide with the critical reversal field, leading to a field window for predictable core reversal.

  16. Magnetic Properties of Antiferromagnetic Iron Oxyhydroxides

    NASA Astrophysics Data System (ADS)

    Guyodo, Y. J.; Till, J. L.; Lagroix, F.; Bonville, P.; Penn, R. L.; Sainctavit, P.; Carvallo, C.; ona-Nguema, G.; Morin, G.

    2013-12-01

    Weakly magnetic iron oxyhydroxides such as ferrihydrite, lepidocrocite or goethite are commonly found in diverse geological and environmental setting, including ground waters and streams, sediments, soils, or acid mine drainage. These minerals take part in multiple biological and abiological processes, and can evolve to more magnetic phases such as hematite, maghemite, or magnetite. Therefore, they represent key minerals with regard to paleoclimate, paleoenvironmental, and paleomagnetic studies. At this meeting, we will present low temperature magnetic properties acquired on fully characterized synthetic samples. The complex nature of the magnetism of these minerals is revealed by comparing magnetic data with other types of characterizations such as high-resolution transmission electron microscopy or synchrotron X-ray magnetic circular dichroism (XMCD), or by studying the early-stages of solid-state alteration (under oxidizing or reducing atmosphere). In particular, we will present recent results about the presence of ferri-magnetic nano-clusters in lepidocrocite, and about uncompensated magnetic moments in goethite nanoparticles.

  17. A Stable Pentagonal Bipyramidal Dy(III) Single-Ion Magnet with a Record Magnetization Reversal Barrier over 1000 K.

    PubMed

    Liu, Jiang; Chen, Yan-Cong; Liu, Jun-Liang; Vieru, Veacheslav; Ungur, Liviu; Jia, Jian-Hua; Chibotaru, Liviu F; Lan, Yanhua; Wernsdorfer, Wolfgang; Gao, Song; Chen, Xiao-Ming; Tong, Ming-Liang

    2016-04-27

    Single-molecule magnets (SMMs) with a large spin reversal barrier have been recognized to exhibit slow magnetic relaxation that can lead to a magnetic hysteresis loop. Synthesis of highly stable SMMs with both large energy barriers and significantly slow relaxation times is challenging. Here, we report two highly stable and neutral Dy(III) classical coordination compounds with pentagonal bipyramidal local geometry that exhibit SMM behavior. Weak intermolecular interactions in the undiluted single crystals are first observed for mononuclear lanthanide SMMs by micro-SQUID measurements. The investigation of magnetic relaxation reveals the thermally activated quantum tunneling of magnetization through the third excited Kramers doublet, owing to the increased axial magnetic anisotropy and weaker transverse magnetic anisotropy. As a result, pronounced magnetic hysteresis loops up to 14 K are observed, and the effective energy barrier (Ueff = 1025 K) for relaxation of magnetization reached a breakthrough among the SMMs. PMID:27054904

  18. A Stable Pentagonal Bipyramidal Dy(III) Single-Ion Magnet with a Record Magnetization Reversal Barrier over 1000 K.

    PubMed

    Liu, Jiang; Chen, Yan-Cong; Liu, Jun-Liang; Vieru, Veacheslav; Ungur, Liviu; Jia, Jian-Hua; Chibotaru, Liviu F; Lan, Yanhua; Wernsdorfer, Wolfgang; Gao, Song; Chen, Xiao-Ming; Tong, Ming-Liang

    2016-04-27

    Single-molecule magnets (SMMs) with a large spin reversal barrier have been recognized to exhibit slow magnetic relaxation that can lead to a magnetic hysteresis loop. Synthesis of highly stable SMMs with both large energy barriers and significantly slow relaxation times is challenging. Here, we report two highly stable and neutral Dy(III) classical coordination compounds with pentagonal bipyramidal local geometry that exhibit SMM behavior. Weak intermolecular interactions in the undiluted single crystals are first observed for mononuclear lanthanide SMMs by micro-SQUID measurements. The investigation of magnetic relaxation reveals the thermally activated quantum tunneling of magnetization through the third excited Kramers doublet, owing to the increased axial magnetic anisotropy and weaker transverse magnetic anisotropy. As a result, pronounced magnetic hysteresis loops up to 14 K are observed, and the effective energy barrier (Ueff = 1025 K) for relaxation of magnetization reached a breakthrough among the SMMs.

  19. Glucose biosensor based on multisegment nanowires exhibiting reversible magnetic control.

    PubMed

    Gerola, Gislaine P; Takahashi, Giovanna S; Perez, Geraldo G; Recco, Lucas C; Pedrosa, Valber A

    2014-11-01

    We describe the amperometric detection of glucose using oriented nanowires with magnetic switching of the bioelectrochemical process. The fabrication process of the nanowires was prepared through controlled nucleation and growth during a stepwise electrochemical deposition, and it was characterized using scanning electron microscopy. Cyclic voltammetry and amperometry were used to study the magnetoswitchable property; this control was accomplished by changing the surface orientation of nanowires. Under the optimal condition, the amperometric response was also linear up to a glucose concentration of 0.1-16.0 mmol L(-1) with a sensitivity of 81 μA mM(-1). The detection limit was estimated for 4.8×10(-8) mol L(-1), defined from a signal/noise ratio of 3. It also exhibits good reproducibility and high selectivity with insignificant interference from ascorbic acid, acetoaminophen, and uric acid. The resulting biosensor was applied to detect the blood sugar in human serum samples without any pretreatment, and the results were comparatively in agreement with the clinical assay. PMID:25127595

  20. Glucose biosensor based on multisegment nanowires exhibiting reversible magnetic control.

    PubMed

    Gerola, Gislaine P; Takahashi, Giovanna S; Perez, Geraldo G; Recco, Lucas C; Pedrosa, Valber A

    2014-11-01

    We describe the amperometric detection of glucose using oriented nanowires with magnetic switching of the bioelectrochemical process. The fabrication process of the nanowires was prepared through controlled nucleation and growth during a stepwise electrochemical deposition, and it was characterized using scanning electron microscopy. Cyclic voltammetry and amperometry were used to study the magnetoswitchable property; this control was accomplished by changing the surface orientation of nanowires. Under the optimal condition, the amperometric response was also linear up to a glucose concentration of 0.1-16.0 mmol L(-1) with a sensitivity of 81 μA mM(-1). The detection limit was estimated for 4.8×10(-8) mol L(-1), defined from a signal/noise ratio of 3. It also exhibits good reproducibility and high selectivity with insignificant interference from ascorbic acid, acetoaminophen, and uric acid. The resulting biosensor was applied to detect the blood sugar in human serum samples without any pretreatment, and the results were comparatively in agreement with the clinical assay.

  1. Temperature-Induced Magnetization Reversal in the Mn^{3+}-Doped SmCrO3

    NASA Astrophysics Data System (ADS)

    Wu, Yuying; Xu, Jian; Xia, Zhengcai

    2016-04-01

    The temperature dependence of dc magnetization is investigated for the rare earth chromites SmCrO3 and the doped compound SmCr_{0.9}Mn_{0.1}O3. Different from the magnetization behavior of SmCrO3, temperature-induced magnetization reversals are observed in the Mn^{3+}-doped compound. Moreover, low-temperature isothermal magnetization measurement indicates the magnetic ground state of SmCr_{0.9}Mn_{0.1}O3 to be antiferromagnetic with a spin canting. The field-cooling magnetic hysteresis loop reveals that an exchange bias (EB) phenomenon is present in the sample. The reversal of magnetization and the corresponding EB field is discussed on the basis of the competitive interaction between the antiferromagnetically coupled Cr-rich clusters and Cr-Mn ordered clusters.

  2. Magnetic properties of ultrathin tetragonal Heusler D022-Mn3Ge perpendicular-magnetized films

    NASA Astrophysics Data System (ADS)

    Sugihara, A.; Suzuki, K. Z.; Miyazaki, T.; Mizukami, S.

    2015-05-01

    We investigated the crystal structure and magnetic properties of Manganese-germanium (Mn3Ge) films having the tetragonal D022 structure, with varied thicknesses (5-130 nm) prepared on chromium (Cr)-buffered single crystal MgO(001) substrates. A crystal lattice elongation in the in-plane direction, induced by the lattice mismatch between the D022-Mn3Ge and the Cr buffer layer, increased with decreasing thickness of the D022-Mn3Ge layer. The films exhibited clear magnetic hysteresis loops with a squareness ratio close to unity, and a step-like magnetization reversal even at a 5-nm thickness under an external field perpendicular to the film's plane. The uniaxial magnetic anisotropy constant of the films showed a reduction to less than 10 Merg/cm3 in the small thickness range (≤20 nm), likely due to the crystal lattice elongation in the in-plane direction.

  3. Reentrant reversible remanent magnetization in superconducting submicron YBaCuO particles

    NASA Astrophysics Data System (ADS)

    Blinov, E. V.; Laiho, R.; Lyublinsky, A. G.; Lähderanta, E.; Traito, K. B.

    1999-05-01

    Reversible properties of the remanent magnetic moment, Mrem, in superconducting submicron- and micron-size Y-Ba-Cu-O particles and thin films are investigated with a SQUID magnetometer. In micron-size particles and thin films a monotonic increase of Mrem was observed when decreasing the temperature. In submicron particles, the same monotonic behaviour is observed at first but at low temperatures an unusual reentrant behaviour was found: Mrem decreased when cooling the sample below 6 K. This phenomenon is independent of the direction of the thermal cycle. Possible mechanisms of this effect, such as midgap states in the quasiparticle excitation spectrum and defect-induced localization of Cooper pairs, are discussed.

  4. Electric field controlled reversible magnetic anisotropy switching studied by spin rectification

    SciTech Connect

    Zhou, Hengan; Fan, Xiaolong Wang, Fenglong; Jiang, Changjun; Rao, Jinwei; Zhao, Xiaobing; Xue, Desheng; Gui, Y. S.; Hu, C.-M.

    2014-03-10

    In this letter, spin rectification was used to study the electric field controlled dynamic magnetic properties of the multiferroic composite which is a Co stripe with induced in-plane anisotropy deposited onto a Pb(Mg{sub 1∕3}Nb{sub 2∕3})O{sub 3}-PbTiO{sub 3} substrate. Due to the coupling between piezoelectric and magnetoelastic effects, a reversible in-plane anisotropy switching has been realized by varying the history of the applied electric field. This merit results from the electric hysteresis of the polarization in the nonlinear piezoelectric regime, which has been proved by a butterfly type electric field dependence of the in-plane anisotropy field. Moreover, the electric field dependent effective demagnetization field and linewidth have been observed at the same time.

  5. Development of Field-Reversed Configuration Plasma Gun Formation Techniques for Magnetized Target Fusion

    NASA Astrophysics Data System (ADS)

    Lynn, Alan; Gilmore, Mark; Wynkoop, Tyler; Intrator, Thomas; Weber, Thomas

    2012-10-01

    Magnetized Target Fusion (MTF) is an innovative approach for a relatively fast and cheap path to the production of fusion energy that utilizes magnetic confinement to assist in the compression of a hot plasma to thermonuclear conditions by an external driver. Los Alamos National Laboratory (LANL) is currently pursing demonstration of the MTF concept via compression of an FRC (field-reversed configuration) plasma by a metal liner z-pinch in conjunction with the Air Force Research Laboratory in Albuquerque, NM. A key physics issue for the FRC as an MTF target lies in the initial pre-ionization (PI) stage. The PI formation process determines the amount of magnetic flux that can be trapped to form the FRC. This trapped flux plays an important role in the FRC's final equilibrium, transport, and stability properties. It also provides the route to greatest potential gains in FRC lifetime, which is essential to provide enough time to translate and compress the FRC effectively. In conjunction with LANL we plan to test and characterize a new system to improve the initial PI plasma formation. This system will use an array of plasma guns to form the initial plasma. Initial characterization of the plasma gun behavior will be presented.

  6. Magnetic properties of ground-state mesons

    NASA Astrophysics Data System (ADS)

    Šimonis, V.

    2016-04-01

    Starting with the bag model a method for the study of the magnetic properties (magnetic moments, magnetic dipole transition widths) of ground-state mesons is developed. We calculate the M1 transition moments and use them subsequently to estimate the corresponding decay widths. These are compared with experimental data, where available, and with the results obtained in other approaches. Finally, we give the predictions for the static magnetic moments of all ground-state vector mesons including those containing heavy quarks. We have a good agreement with experimental data for the M1 decay rates of light as well as heavy mesons. Therefore, we expect our predictions for the static magnetic properties ( i.e., usual magnetic moments) to be of sufficiently high quality, too.

  7. Interactions and reversal-field memory in complex magnetic nanowire arrays

    NASA Astrophysics Data System (ADS)

    Rotaru, Aurelian; Lim, Jin-Hee; Lenormand, Denny; Diaconu, Andrei; Wiley, John. B.; Postolache, Petronel; Stancu, Alexandru; Spinu, Leonard

    2011-10-01

    Interactions and magnetization reversal of Ni nanowire arrays have been investigated by the first-order reversal curve (FORC) method. Several series of samples with controlled spatial distribution were considered including simple wires of different lengths and diameters (70 and 110 nm) and complex wires with a single modulated diameter along their length. Subtle features of magnetic interactions are revealed through a quantitative analysis of the local interaction field profile distributions obtained from the FORC method. In addition, the FORC analysis indicates that the nanowire systems with a mean diameter of 70 nm appear to be organized in symmetric clusters indicative of a reversal-field memory effect.

  8. Magnetization reversal induced by in-plane current in Ta/CoFeB/MgO structures with perpendicular magnetic easy axis

    SciTech Connect

    Zhang, C.; Yamanouchi, M. Ikeda, S.; Sato, H.; Fukami, S.; Matsukura, F.; Ohno, H.

    2014-05-07

    We investigate in-plane current-induced magnetization reversal under an in-plane magnetic field in Hall bar shaped devices composed of Ta/CoFeB/MgO structures with perpendicular magnetic easy axis. The observed relationship between the directions of current and magnetization switching and Ta thickness dependence of magnetization switching current are accordance with those for magnetization reversal by spin transfer torque originated from the spin Hall effect in the Ta layer.

  9. Low-Noise YBa2Cu3O7 Nano-SQUIDs for Performing Magnetization-Reversal Measurements on Magnetic Nanoparticles

    NASA Astrophysics Data System (ADS)

    Schwarz, T.; Wölbing, R.; Reiche, C. F.; Müller, B.; Martínez-Pérez, M. J.; Mühl, T.; Büchner, B.; Kleiner, R.; Koelle, D.

    2015-04-01

    We fabricate YBa2Cu3O7 (YBCO) direct-current nano- superconducting quantum-interference devices (nano-SQUIDs) based on grain-boundary Josephson junctions by focused-ion-beam patterning. Characterization of electric transport and noise properties at 4.2 K in a magnetically shielded environment yields a very small inductance L of a few pH for an optimized device geometry. This, in turn, results in very low values of flux noise <50 n Φ0/Hz1 /2 in the thermal white-noise limit, which yields spin sensitivities of a few μB/Hz1 /2 (Φ0 is the magnetic flux quantum, and μB is the Bohr magneton). We observe frequency-dependent excess noise up to 7 MHz, which can be eliminated only partially by bias reversal readout. This behavior indicates the presence of fluctuators of unknown origin, possibly related to defect-induced spins in the SrTiO3 substrate. We demonstrate the potential of using YBCO nano-SQUIDs for the investigation of small spin systems, by placing a 39-nm-diameter Fe nanowire encapsulated in a carbon nanotube on top of a nonoptimized YBCO nano-SQUID and by measuring the magnetization reversal of the Fe nanowire via the change of magnetic flux coupled to the nano-SQUID. The measured flux signals upon magnetization reversal of the Fe nanowire are in very good agreement with estimated values, and the determined switching fields indicate magnetization reversal of the nanowire via curling mode.

  10. Microstructure and magnetic properties of MnZn-ferrite

    SciTech Connect

    Lin, I.N.

    1982-12-01

    Grain boundaries in MnZn-ferrites have been characterized and their effects on the magnetic and electrical properties have been investigated. Addition of CaO into MnZn-ferrite materials leads to the formation of secondary phases along the grain boundaries. It is concluded that the Ca addition does not produce beneficial effects on the electrical properties but only leads to a detrimental influence on the magnetic properties. Other microstructural features such as secondary phases and stacking faults will also affect the domain wall dynanics. They not only retard the domain wall motion but can also act as nucleation sites for domains of reverse magnetization. Controlled-atmosphere annealing improves drastically the apparent resistivity of the sintered MnZn-ferrites through the reduction of ferrous ions content but degrades the magnetic permeability. Control of the oxygen partial pressure at an earlier stage of processing rather than post fabrication annealing is needed in order to raise the intrinsic electrical resistivity of the bulk materials by reducing ferrous ion concentration without affecting the magnetic permeability detrimentally. 145 references, 20 figures.

  11. A field-reversed magnetic configuration and applications of high-temperature FRC plasma

    SciTech Connect

    Ryzhkov, S. V.

    2011-12-15

    As applied to a tokomak, a magnetic trap for confinement of a plasma with an inverted field or a magnetic field reversed configuration (FRC) is one of the most promising alternatives of the systems with high {beta}. A brief review of the latest data on FRC and potential directions of using such configurations in addition to energy generation in thermonuclear reactors (TNRs) is proposed.

  12. Magnetic-field-induced ferroelectric polarization reversal in magnetoelectric composites revealed by piezoresponse force microscopy

    NASA Astrophysics Data System (ADS)

    Miao, Hongchen; Zhou, Xilong; Dong, Shuxiang; Luo, Haosu; Li, Faxin

    2014-07-01

    Controlling electric polarization (or magnetization) in multiferroic materials with external magnetic fields (or electric fields) is very important for fundamental physics and spintronic devices. Although there has been some progress on magnetic-field-induced polarization reversal in single-phase multiferroics, such behavior has so far never been realized in composites. Here we show that it is possible to reverse ferroelectric polarization using magnetic fields in a bilayer Terfenol-D/PMN-33%PT composite. We realized this by ferroelectric domain imaging using piezoresponse force microscopy (PFM) under applied magnetic field loading. The internal electric field caused by the magnetoelectric (ME) effect in the PMN-PT crystal is considered as the driving force for the 180° polarization switching, and its existence is verified by switching spectroscopy PFM testing under a series of external magnetic fields. A quantitative method is further suggested to estimate the local ME coefficient based on the switching spectroscopy PFM testing results.

  13. Magnetic-field-induced ferroelectric polarization reversal in magnetoelectric composites revealed by piezoresponse force microscopy.

    PubMed

    Miao, Hongchen; Zhou, Xilong; Dong, Shuxiang; Luo, Haosu; Li, Faxin

    2014-08-01

    Controlling electric polarization (or magnetization) in multiferroic materials with external magnetic fields (or electric fields) is very important for fundamental physics and spintronic devices. Although there has been some progress on magnetic-field-induced polarization reversal in single-phase multiferroics, such behavior has so far never been realized in composites. Here we show that it is possible to reverse ferroelectric polarization using magnetic fields in a bilayer Terfenol-D/PMN-33%PT composite. We realized this by ferroelectric domain imaging using piezoresponse force microscopy (PFM) under applied magnetic field loading. The internal electric field caused by the magnetoelectric (ME) effect in the PMN-PT crystal is considered as the driving force for the 180° polarization switching, and its existence is verified by switching spectroscopy PFM testing under a series of external magnetic fields. A quantitative method is further suggested to estimate the local ME coefficient based on the switching spectroscopy PFM testing results. PMID:24953042

  14. Antiphase domains and reverse thermoremanent magnetism in ilmenite-hematite minerals

    USGS Publications Warehouse

    Lawson, C.A.; Nord, G.L.; Dowty, Eric; Hargraves, R.B.

    1981-01-01

    Examination of synthetic ilmenite-hematite samples by transmission electron microscopy has for the first time revealed the presence of well-defined antiphase domains and antiphase domain boundaries in this mineral system. Samples quenched from 1300??C have a high density of domain boundaries, whereas samples quenched from 900??C have a much lower density. Only the high-temperature samples acquire reverse thermoremanent magnetism when cooled in an applied magnetic field. The presence of a high density of domain boundaries seems to be a necessary condition for the acquisition of reverse thermoremanent magnetism.

  15. Hanle effect as a magnetic diagnostic for field-reversed configuration plasmas

    NASA Astrophysics Data System (ADS)

    Gupta, Deepak K.

    2016-11-01

    Hanle effect is presented as a low magnetic-field diagnostic for field-reversed configuration (FRC) plasmas. The non-perturbative technique is capable of measuring not only magnetic-field profile and direction but also field-null position and its shape. Conditions and configurations for the measurement are discussed. The technique is applicable to other low magnetic-field laboratory plasmas, e.g., magnetic-cusps, where measurements of low field are desirable, and it may also be extended to measure the two-dimensional vector magnetic-field.

  16. Stochastic reversal dynamics of two interacting magnetic dipoles: A simple model experiment.

    PubMed

    Plihon, Nicolas; Miralles, Sophie; Bourgoin, Mickael; Pinton, Jean-François

    2016-07-01

    We report an experimental study of the dynamics of two coupled magnetic dipoles. The experiment consists in two coplanar permanent disk magnets separated by a distance d, each allowed to rotate on a fixed parallel axis-each magnet's axis being perpendicular to its dipolar moment vector. A torque of adjustable strength can be externally applied to one of the magnets, the other magnet being free. The driving torque may be time-independent or temporally fluctuating. We study the influence of the parameters of the driving torque on the dynamics of the coupled system, in particular the emergence of dynamical regimes such as stochastic reversals. We report transitions between stationary and stochastic reversal regimes. All the observed features can be understood by a simple mechanical dynamical model. The transition between statistically stationary regimes and reversals is explained introducing an effective potential energy incorporating both the coupling between magnets and the external driving. Relations between this simple experimental model with macroscopic models of magnetic spin coupling, as well as with chaotic reversals of turbulent dynamos, are discussed. PMID:27575140

  17. Preparation and characterization of supported magnetic nanoparticles prepared by reverse micelles

    PubMed Central

    Han, Luyang; Biskupek, Johannes; Kaiser, Ute; Ziemann, Paul

    2010-01-01

    Summary Monatomic (Fe, Co) and bimetallic (FePt and CoPt) nanoparticles were prepared by exploiting the self-organization of precursor loaded reverse micelles. Achievements and limitations of the preparation approach are critically discussed. We show that self-assembled metallic nanoparticles can be prepared with diameters d = 2–12 nm and interparticle distances D = 20–140 nm on various substrates. Structural, electronic and magnetic properties of the particle arrays were characterized by several techniques to give a comprehensive view of the high quality of the method. For Co nanoparticles, it is demonstrated that magnetostatic interactions can be neglected for distances which are at least 6 times larger than the particle diameter. Focus is placed on FePt alloy nanoparticles which show a huge magnetic anisotropy in the L10 phase, however, this is still less by a factor of 3–4 when compared to the anisotropy of the bulk counterpart. A similar observation was also found for CoPt nanoparticles (NPs). These results are related to imperfect crystal structures as revealed by HRTEM as well as to compositional distributions of the prepared particles. Interestingly, the results demonstrate that the averaged effective magnetic anisotropy of FePt nanoparticles does not strongly depend on size. Consequently, magnetization stability should scale linearly with the volume of the NPs and give rise to a critical value for stability at ambient temperature. Indeed, for diameters above 6 nm such stability is observed for the current FePt and CoPt NPs. Finally, the long-term conservation of nanoparticles by Au photoseeding is presented. PMID:21977392

  18. Sudden motility reversal indicates sensing of magnetic field gradients in Magnetospirillum magneticum AMB-1 strain

    PubMed Central

    González, Lina M; Ruder, Warren C; Mitchell, Aaron P; Messner, William C; LeDuc, Philip R

    2015-01-01

    Many motile unicellular organisms have evolved specialized behaviors for detecting and responding to environmental cues such as chemical gradients (chemotaxis) and oxygen gradients (aerotaxis). Magnetotaxis is found in magnetotactic bacteria and it is defined as the passive alignment of these cells to the geomagnetic field along with active swimming. Herein we show that Magnetospirillum magneticum (AMB-1) show a unique set of responses that indicates they sense and respond not only to the direction of magnetic fields by aligning and swimming, but also to changes in the magnetic field or magnetic field gradients. We present data showing that AMB-1 cells exhibit sudden motility reversals when we impose them to local magnetic field gradients. Our system employs permalloy (Ni80Fe20) islands to curve and diverge the magnetic field lines emanating from our custom-designed Helmholtz coils in the vicinity of the islands (creating a drop in the field across the islands). The three distinct movements we have observed as they approach the permalloy islands are: unidirectional, single reverse and double reverse. Our findings indicate that these reverse movements occur in response to magnetic field gradients. In addition, using a permanent magnet we found further evidence that supports this claim. Motile AMB-1 cells swim away from the north and south poles of a permanent magnet when the magnet is positioned less than ∼30 mm from the droplet of cells. All together, these results indicate previously unknown response capabilities arising from the magnetic sensing systems of AMB-1 cells. These responses could enable them to cope with magnetic disturbances that could in turn potentially inhibit their efficient search for nutrients. PMID:25478682

  19. Sudden motility reversal indicates sensing of magnetic field gradients in Magnetospirillum magneticum AMB-1 strain.

    PubMed

    González, Lina M; Ruder, Warren C; Mitchell, Aaron P; Messner, William C; LeDuc, Philip R

    2015-06-01

    Many motile unicellular organisms have evolved specialized behaviors for detecting and responding to environmental cues such as chemical gradients (chemotaxis) and oxygen gradients (aerotaxis). Magnetotaxis is found in magnetotactic bacteria and it is defined as the passive alignment of these cells to the geomagnetic field along with active swimming. Herein we show that Magnetospirillum magneticum (AMB-1) show a unique set of responses that indicates they sense and respond not only to the direction of magnetic fields by aligning and swimming, but also to changes in the magnetic field or magnetic field gradients. We present data showing that AMB-1 cells exhibit sudden motility reversals when we impose them to local magnetic field gradients. Our system employs permalloy (Ni(80)Fe(20)) islands to curve and diverge the magnetic field lines emanating from our custom-designed Helmholtz coils in the vicinity of the islands (creating a drop in the field across the islands). The three distinct movements we have observed as they approach the permalloy islands are: unidirectional, single reverse and double reverse. Our findings indicate that these reverse movements occur in response to magnetic field gradients. In addition, using a permanent magnet we found further evidence that supports this claim. Motile AMB-1 cells swim away from the north and south poles of a permanent magnet when the magnet is positioned less than ∼30 mm from the droplet of cells. All together, these results indicate previously unknown response capabilities arising from the magnetic sensing systems of AMB-1 cells. These responses could enable them to cope with magnetic disturbances that could in turn potentially inhibit their efficient search for nutrients. PMID:25478682

  20. Sudden motility reversal indicates sensing of magnetic field gradients in Magnetospirillum magneticum AMB-1 strain.

    PubMed

    González, Lina M; Ruder, Warren C; Mitchell, Aaron P; Messner, William C; LeDuc, Philip R

    2015-06-01

    Many motile unicellular organisms have evolved specialized behaviors for detecting and responding to environmental cues such as chemical gradients (chemotaxis) and oxygen gradients (aerotaxis). Magnetotaxis is found in magnetotactic bacteria and it is defined as the passive alignment of these cells to the geomagnetic field along with active swimming. Herein we show that Magnetospirillum magneticum (AMB-1) show a unique set of responses that indicates they sense and respond not only to the direction of magnetic fields by aligning and swimming, but also to changes in the magnetic field or magnetic field gradients. We present data showing that AMB-1 cells exhibit sudden motility reversals when we impose them to local magnetic field gradients. Our system employs permalloy (Ni(80)Fe(20)) islands to curve and diverge the magnetic field lines emanating from our custom-designed Helmholtz coils in the vicinity of the islands (creating a drop in the field across the islands). The three distinct movements we have observed as they approach the permalloy islands are: unidirectional, single reverse and double reverse. Our findings indicate that these reverse movements occur in response to magnetic field gradients. In addition, using a permanent magnet we found further evidence that supports this claim. Motile AMB-1 cells swim away from the north and south poles of a permanent magnet when the magnet is positioned less than ∼30 mm from the droplet of cells. All together, these results indicate previously unknown response capabilities arising from the magnetic sensing systems of AMB-1 cells. These responses could enable them to cope with magnetic disturbances that could in turn potentially inhibit their efficient search for nutrients.

  1. Crystal field and magnetic properties

    NASA Technical Reports Server (NTRS)

    Flood, D. J.

    1977-01-01

    Magnetization and magnetic susceptibility measurements have been made in the temperature range 1.3 to 4.2 K on powdered samples of ErH3. The susceptibility exhibits Curie-Weiss behavior from 4.2 to 2 K, and intercepts the negative temperature axis at theta = 1.05 + or - 0.05 K, indicating that the material is antiferromagnetic. The low field effective moment is 6.77 + or - 0.27 Bohr magnetons per ion. The magnetization exhibits a temperature independent contribution, the slope of which is (5 + or - 1.2) x 10 to the -6th Weber m/kg Tesla. The saturation moment is 3.84 + or - 1 - 0.15 Bohr magnetons per ion. The results can be qualitatively explained by the effects of crystal fields on the magnetic ions. No definitive assignment of a crystal field ground state can be given, nor can a clear choice between cubically or hexagonally symmetric crystal fields be made. For hexagonal symmetry, the first excited state is estimated to be 86 to 100 K above the ground state. For cubic symmetry, the splitting is on the order of 160 to 180 K.

  2. Magnetic field induced flow pattern reversal in a ferrofluidic Taylor-Couette system

    PubMed Central

    Altmeyer, Sebastian; Do, Younghae; Lai, Ying-Cheng

    2015-01-01

    We investigate the dynamics of ferrofluidic wavy vortex flows in the counter-rotating Taylor-Couette system, with a focus on wavy flows with a mixture of the dominant azimuthal modes. Without external magnetic field flows are stable and pro-grade with respect to the rotation of the inner cylinder. More complex behaviors can arise when an axial or a transverse magnetic field is applied. Depending on the direction and strength of the field, multi-stable wavy states and bifurcations can occur. We uncover the phenomenon of flow pattern reversal as the strength of the magnetic field is increased through a critical value. In between the regimes of pro-grade and retrograde flow rotations, standing waves with zero angular velocities can emerge. A striking finding is that, under a transverse magnetic field, a second reversal in the flow pattern direction can occur, where the flow pattern evolves into pro-grade rotation again from a retrograde state. Flow reversal is relevant to intriguing phenomena in nature such as geomagnetic reversal. Our results suggest that, in ferrofluids, flow pattern reversal can be induced by varying a magnetic field in a controlled manner, which can be realized in laboratory experiments with potential applications in the development of modern fluid devices. PMID:26687638

  3. Magnetic field induced flow pattern reversal in a ferrofluidic Taylor-Couette system.

    PubMed

    Altmeyer, Sebastian; Do, Younghae; Lai, Ying-Cheng

    2015-01-01

    We investigate the dynamics of ferrofluidic wavy vortex flows in the counter-rotating Taylor-Couette system, with a focus on wavy flows with a mixture of the dominant azimuthal modes. Without external magnetic field flows are stable and pro-grade with respect to the rotation of the inner cylinder. More complex behaviors can arise when an axial or a transverse magnetic field is applied. Depending on the direction and strength of the field, multi-stable wavy states and bifurcations can occur. We uncover the phenomenon of flow pattern reversal as the strength of the magnetic field is increased through a critical value. In between the regimes of pro-grade and retrograde flow rotations, standing waves with zero angular velocities can emerge. A striking finding is that, under a transverse magnetic field, a second reversal in the flow pattern direction can occur, where the flow pattern evolves into pro-grade rotation again from a retrograde state. Flow reversal is relevant to intriguing phenomena in nature such as geomagnetic reversal. Our results suggest that, in ferrofluids, flow pattern reversal can be induced by varying a magnetic field in a controlled manner, which can be realized in laboratory experiments with potential applications in the development of modern fluid devices. PMID:26687638

  4. Magnetic field induced flow pattern reversal in a ferrofluidic Taylor-Couette system

    NASA Astrophysics Data System (ADS)

    Altmeyer, Sebastian; Do, Younghae; Lai, Ying-Cheng

    2015-12-01

    We investigate the dynamics of ferrofluidic wavy vortex flows in the counter-rotating Taylor-Couette system, with a focus on wavy flows with a mixture of the dominant azimuthal modes. Without external magnetic field flows are stable and pro-grade with respect to the rotation of the inner cylinder. More complex behaviors can arise when an axial or a transverse magnetic field is applied. Depending on the direction and strength of the field, multi-stable wavy states and bifurcations can occur. We uncover the phenomenon of flow pattern reversal as the strength of the magnetic field is increased through a critical value. In between the regimes of pro-grade and retrograde flow rotations, standing waves with zero angular velocities can emerge. A striking finding is that, under a transverse magnetic field, a second reversal in the flow pattern direction can occur, where the flow pattern evolves into pro-grade rotation again from a retrograde state. Flow reversal is relevant to intriguing phenomena in nature such as geomagnetic reversal. Our results suggest that, in ferrofluids, flow pattern reversal can be induced by varying a magnetic field in a controlled manner, which can be realized in laboratory experiments with potential applications in the development of modern fluid devices.

  5. Plasmonic enhancement of ultrafast all-optical magnetization reversal

    NASA Astrophysics Data System (ADS)

    Kochergin, Vladimir; Neely, Lauren N.; Allin, Leigh J.; Kochergin, Eugene V.; Wang, Kang L.

    2011-10-01

    Ultrafast all optical magnetization switching in GdFeCo layers on the basis of Inverse Faraday Effect (IFE) was demonstrated recently and suggested as a possible path toward next generation magnetic data storage medium with much faster writing time. However, to date, the demonstrations of ultrafast all-optical magnetization switching were performed with powerful femtosecond lasers, hardly useful for practical applications in data storage and data processing. Here we show that utilization of IFE enhancement in plasmonic nanostructures enables fast all-optical magnetization switching with smaller/cheaper laser sources with longer pulse durations. Our modeling results predict significant enhancement of IFE around all major types of plasmonic nanostructures for a circularly polarized incident light. Unlike the IFE in uniform bulk materials, nonzero value of IFE is predicted in plasmonic nanostructures even with a linearly polarized excitation. Experimentally, all-optical magnetization switching at 20 times lower laser fluence and roughly 100 times lower value of laser fluence/pulse duration ratio is demonstrated in plasmonic samples to verify the model predictions. The path to achieve higher levels of enhancement experimentally is discussed.

  6. Tailoring Magnetic Properties in Bulk Nanostructured Solids

    NASA Astrophysics Data System (ADS)

    Morales, Jason Rolando

    Important magnetic properties and behaviors such as coercivity, remanence, susceptibility, energy product, and exchange coupling can be tailored by controlling the grain size, composition, and density of bulk magnetic materials. At nanometric length scales the grain size plays an increasingly important role since magnetic domain behavior and grain boundary concentration determine bulk magnetic behavior. This has spurred a significant amount of work devoted to developing magnetic materials with nanometric features (thickness, grain/crystallite size, inclusions or shells) in 0D (powder), 1D (wires), and 2D (thin films) materials. Large 3D nanocrystalline materials are more suitable for many applications such as permanent magnets, magneto-optical Faraday isolators etc. Yet there are relatively few successful demonstrations of 3D magnetic materials with nanoscale influenced properties available in the literature. Making dense 3D bulk materials with magnetic nanocrystalline microstructures is a challenge because many traditional densification techniques (HIP, pressureless sintering, etc.) move the microstructure out of the "nano" regime during densification. This dissertation shows that the Current Activated Pressure Assisted Densification (CAPAD) method, also known as spark plasma sintering, can be used to create dense, bulk, magnetic, nanocrystalline solids with varied compositions suited to fit many applications. The results of my research will first show important implications for the use of CAPAD for the production of exchange-coupled nanocomposite magnets. Decreases in grain size were shown to have a significant role in increasing the magnitude of exchange bias. Second, preferentially ordered bulk magnetic materials were produced with highly anisotropic material properties. The ordered microstructure resulted in changing magnetic property magnitudes (ex. change in coercivity by almost 10x) depending on the relative orientation (0° vs. 90°) of an externally

  7. Influence of carbon doping on the reversible magnetization of MgB 2 single crystals

    NASA Astrophysics Data System (ADS)

    Eisterer, M.; Krutzler, C.; Zehetmayer, M.; Weber, H. W.; Kazakov, S. M.; Karpinski, J.

    2007-09-01

    The reversible magnetization of Mg(B1-xCx)2 single crystals with varying carbon content (x = 0-0.095) was measured by SQUID magnetometry. It was found to be strongly influenced by the two-band character of this material. At low magnetic fields charge carriers of both bands contribute to superconductivity and to diamagnetism. At high fields the π-band is suppressed and the σ-band mainly determines the magnetization. This allows us to extract information on both bands by analyzing the reversible magnetization in terms of two band Ginzburg-Landau (GL) theory. The "intrinsic" magnetic penetration increases in both bands with increasing carbon content, but the σ-band remains crucial for the upper critical field. Changes in the field dependence of the resulting "effective" penetration depth by carbon doping are discussed.

  8. Study on the pulse reverse electrodeposition of Fe-nano-Si composite coatings in magnetic field

    NASA Astrophysics Data System (ADS)

    Zhong, Yunbo; Zhou, Pengwei; Zhou, Junfeng; Wang, Huai; Fan, Lijun; Dong, Licheng; Zheng, Tianxiang; Shen, Weiwen

    2014-08-01

    Composite iron deposits containing nano-silicon particles were prepared under direct current (DCED) and pulse reverse current electrodeposition (PRED) conditions in the presence of magnetic field. The influences of magnetic field and pulse reverse current on the co-deposition of silicon particles as well as the surface morphology of coatings were investigated respectively. Results showed that PRED regime exhibits fewer incorporated silicon particles than those obtained under DCED condition when no magnetic field was applied. Under the influence of magnetic field, the silicon particles of coatings increased significantly, meanwhile, many projecting deposits named “mountain ranges” appeared on the surface of coatings. However, the numbers of “mountain ranges” showed a trend of reduce with increasing the pulse frequency under magnetic field and therefore the surface morphology of coatings became more smooth and flat.

  9. Magnetic properties of the Esquel Pallasite

    NASA Astrophysics Data System (ADS)

    Erickson, A. M.; Tarduno, J. A.; Cottrell, R. D.

    2009-12-01

    Pallasites are stony-iron meteorites consisting mainly of olivine crystals suspended in an iron-nickel matrix. One hypothesis holds that pallasites are formed from the intrusion of a liquid iron-nickel core into the solid silicate mantle of a parent body. The magnetic properties of the olivine crystals could help provide insight into the veracity of this explanation. The olivine crystals may contain magnetic inclusions that record useful information regarding magnetic fields present in the parent body. The best recorders of magnetic information are single domain in nature; domain structure of magnetic inclusions can be examined by recording their hysteresis properties. Olivine crystals were separated from a sample of the Esquel pallasite. Crystal fragments were often stained or coated with non-olivine minerals, which required cleaning to remove. An Alternating Gradient Force Magnetometer (AGFM) was used to measure magnetic hysteresis properties, and a Superconducting Quantum Interface Device Cryogenic Rock Magnetometer was used to measure the natural remanent magnetization of the samples. Preliminary data indicate single domain carriers in select olivine crystals that carry records of strong ancient fields. This is a presentation of preliminary results collected during a summer REU at the University of Rochester.

  10. Geometry Dependence of Magnetization Reversal in Nanocomposite Alloys

    SciTech Connect

    Skomski, R; Manchanda, P; Takeuchi, I; Cui, J

    2014-05-31

    The geometrical optimization of aligned hard-soft permanent-magnet nanocomposites is investigated by model calculations. Considered criteria are the shapes of the soft and c-axis-aligned hard phases, the packing fraction of the soft phase, and magnetostatic interactions. Taking into account that the energy product is enhanced via the volume fraction of the soft phase, subject to maintaining coercivity, we find that the best structures are soft-magnetic cubes as well as long rods with a square cross section. Comparing embedded soft cubes with embedded soft spheres of the same size, our nucleation-field analysis shows that the volume fraction of the soft phase is enhanced by 91%, with a coercivity reduction of only 25%. Magnetostatic interactions often but not always deteriorate the permanent-magnet performance, as exemplified by the example of MnBi:FeCo bilayers and multilayers.

  11. Geometry Dependence of Magnetization Reversal in Nanocomposite Alloys

    SciTech Connect

    Skomski, Ralph; Manchanda, Priyanka; Takeuchi, Ichiro; Cui, Jun

    2014-06-11

    The geometrical optimization of aligned hard-soft permanent-magnet nanocomposites is investigated by model calculations. Considered criteria are the shapes of the soft and c-axis-aligned hard phases, the packing fraction of the soft phase, and magnetostatic interactions. Taking into account that the energy product is enhanced via the volume fraction of the soft phase, subject to maintaining coercivity, we find that the best structures are soft-magnetic cubes as well as long rods with a square cross section. Comparing embedded soft cubes with embedded soft spheres of the same size, our nucleation-field analysis shows that the volume fraction of the soft phase is enhanced by 91%, with a coercivity reduction of only 25%. Magnetostatic interactions often but not always deteriorate the permanent-magnet performance, as exemplified by the example of MnBi:FeCo bilayers and multilayers.

  12. Tuning the Magnetic Properties of Nanoparticles

    PubMed Central

    Kolhatkar, Arati G.; Jamison, Andrew C.; Litvinov, Dmitri; Willson, Richard C.; Lee, T. Randall

    2013-01-01

    The tremendous interest in magnetic nanoparticles (MNPs) is reflected in published research that ranges from novel methods of synthesis of unique nanoparticle shapes and composite structures to a large number of MNP characterization techniques, and finally to their use in many biomedical and nanotechnology-based applications. The knowledge gained from this vast body of research can be made more useful if we organize the associated results to correlate key magnetic properties with the parameters that influence them. Tuning these properties of MNPs will allow us to tailor nanoparticles for specific applications, thus increasing their effectiveness. The complex magnetic behavior exhibited by MNPs is governed by many factors; these factors can either improve or adversely affect the desired magnetic properties. In this report, we have outlined a matrix of parameters that can be varied to tune the magnetic properties of nanoparticles. For practical utility, this review focuses on the effect of size, shape, composition, and shell-core structure on saturation magnetization, coercivity, blocking temperature, and relaxation time. PMID:23912237

  13. Direct real-space observation of nearly stochastic behavior in magnetization reversal process on a nanoscale

    SciTech Connect

    Im, M.-Y.; Kim, D.-H.; Lee, K.-D.; Fischer, P.; Shin, S.-C.

    2007-06-01

    We report a non-deterministic nature in the magnetization reversal of nanograins of CoCrPt alloy film. Magnetization reversal process of CoCrPt alloy film is investigated using high resolution soft X-ray microscopy which provides real space images with a spatial resolution of 15 nm. Domain nucleation sites mostly appear stochastically distributed within repeated hysteretic cycles, where the correlation increases as the strength of the applied magnetic field increases in the descending and ascending branches of the major hysteresis loop. In addition, domain configuration is mostly asymmetric with inversion of an applied magnetic field in the hysteretic cycle. Nanomagnetic simulation considering thermal fluctuations of the magnetic moments of the grains explains the nearly stochastic nature of the domain nucleation behavior observed in CoCrPt alloy film. With the bit size in high-density magnetic recording media approaching nanometer length scale, one of the fundamental and crucial issues is whether the domain nucleation during magnetization reversal process exhibits a deterministic behavior. Repeatability of local domain nucleation and deterministic switching behavior are basic and essential factors for achieving high performance in high-density magnetic recording [1-3]. Most experimental studies on this issue reported so far have been mainly performed by indirect probes through macroscopic hysteresis loop and Barkhausen pattern measurements, which provide the ensemble-average magnetization. Thus, they are inadequate to gain insight into the domain-nucleation behavior on a nanometer length scale during the magnetization reversal process [4-6]. Very recently, coherent X-ray speckle metrology, where the speckle pattern observed in reciprocal space acts as a fingerprint of the domain configurations, was adopted to investigate stochastic behavior in the magnetization reversal of a Co/Pt multilayer film [7,8]. However, no direct observation on the stochastic behavior of

  14. Characterization of the magnetization reversal of perpendicular Nanomagnetic Logic clocked in the ns-range

    NASA Astrophysics Data System (ADS)

    Ziemys, Grazvydas; Trummer, Christian; Gamm, Stephan Breitkreutz-v.; Eichwald, Irina; Schmitt-Landsiedel, Doris; Becherer, Markus

    2016-05-01

    We have investigated the magnetization reversal of fabricated Co/Pt nanomagnets with perpendicular anisotropy within a wide range of magnetic field pulse widths. This experiment covers the pulse lengths from 700 ms to 20 ns. We observed that the commonly used Arrhenius model fits very well the experimental data with a single parameter set for pulse times above 100 ns (tp > 100 ns). However, below 100 ns (tp < 100 ns), a steep increase of the switching field amplitude is observed and the deviation from the Arrhenius model becomes unacceptable. For short pulse times the model can be adjusted by the reversal time term for the dynamic switching field which is only dependent on the pulse amplitude and not on temperature anymore. Precise modeling of the magnetization reversal in the sub-100 ns-range is crucially important to ensure reliable operation in the favored GHz-range as well as to explore and design new kinds of Nanomagnetic Logic circuits and architectures.

  15. Dynamics and efficiency of magnetic vortex circulation reversal

    NASA Astrophysics Data System (ADS)

    Urbánek, Michal; Uhlíř, Vojtěch; Lambert, Charles-Henri; Kan, Jimmy J.; Eibagi, Nasim; VaÅatka, Marek; Flajšman, Lukáš; Kalousek, Radek; Im, Mi-Young; Fischer, Peter; Šikola, Tomáš; Fullerton, Eric E.

    2015-03-01

    Dynamic switching of the vortex circulation in magnetic nanodisks by fast-rising magnetic field pulse requires annihilation of the vortex core at the disk boundary and reforming a new vortex with the opposite sense of circulation. Here we study the influence of pulse parameters on the dynamics and efficiency of the vortex core annihilation in permalloy (Ni80Fe20 ) nanodisks. We use magnetic transmission soft x-ray microscopy to experimentally determine a pulse rise time-pulse amplitude phase diagram for vortex circulation switching and investigate the time-resolved evolution of magnetization in different regions of the phase diagram. The experimental phase diagram is compared with an analytical model based on Thiele's equation describing high-amplitude vortex core motion in a parabolic potential. We find that the analytical model is in good agreement with experimental data for a wide range of disk geometries. From the analytical model and in accordance with our experimental finding we determine the geometrical condition for dynamic vortex core annihilation and pulse parameters needed for the most efficient and fastest circulation switching. The comparison of our experimental results with micromagnetic simulations shows that the micromagnetic simulations of "ideal" disks with diameters larger than ˜250 nm overestimate nonlinearities in susceptibility and eigenfrequency. This overestimation leads to the core polarity switching near the disk boundary, which then in disagreement with experimental findings prevents the core annihilation and circulation switching. We modify the micromagnetic simulations by introducing the "boundary region" of reduced magnetization to simulate the experimentally determined susceptibility and in these modified micromagnetic simulations we are able to reproduce the experimentally observed dynamic vortex core annihilation and circulation switching.

  16. Reconstruction of magnetic domain structure using the reverse Monte Carlo method with an extended Fourier image

    PubMed Central

    Tokii, Maki; Kita, Eiji; Mitsumata, Chiharu; Ono, Kanta; Yanagihara, Hideto

    2015-01-01

    Visualization of the magnetic domain structure is indispensable to the investigation of magnetization processes and the coercivity mechanism. It is necessary to develop a reconstruction method from the reciprocal-space image to the real-space image. For this purpose, it is necessary to solve the problem of missing phase information in the reciprocal-space image. We propose the method of extend Fourier image with mean-value padding to compensate for the phase information. We visualized the magnetic domain structure using the Reverse Monte Carlo method with simulated annealing to accelerate the calculation. With this technique, we demonstrated the restoration of the magnetic domain structure, obtained magnetization and magnetic domain width, and reproduced the characteristic form that constitutes a magnetic domain. PMID:25991875

  17. Using Polar Coronal Hole Area Measurements to Determine the Solar Polar Magnetic Field Reversal in Solar Cycle 24

    NASA Technical Reports Server (NTRS)

    Karna, N.; Webber, S.A. Hess; Pesnell, W.D.

    2014-01-01

    An analysis of solar polar coronal hole (PCH) areas since the launch of the Solar Dynamics Observatory (SDO) shows how the polar regions have evolved during Solar Cycle 24. We present PCH areas from mid-2010 through 2013 using data from the Atmospheric Imager Assembly (AIA) and Helioseismic and Magnetic Imager (HMI) instruments onboard SDO. Our analysis shows that both the northern and southern PCH areas have decreased significantly in size since 2010. Linear fits to the areas derived from the magnetic-field properties indicate that, although the northern hemisphere went through polar-field reversal and reached solar-maximum conditions in mid-2012, the southern hemisphere had not reached solar-maximum conditions in the polar regions by the end of 2013. Our results show that solar-maximum conditions in each hemisphere, as measured by the area of the polar coronal holes and polar magnetic field, will be offset in time.

  18. Magnetic properties of magnetoactive spin clusters

    SciTech Connect

    Khamzin, A. M.; Nigmatullin, R. R.

    2010-01-15

    A simple model is proposed for describing magnetic properties of magnetoactive nanoclusters, which permits exact analytic solution. Exact expressions are obtained for thermodynamic characteristics of the model, which hold in the entire range of temperatures, magnetic fields, and interaction parameters. It is found that in the case of easy-axis anisotropy, the field dependence of magnetization of a nanocluster consisting of N particles with a spin of 1/2 has [N/2] fractional plateaus ([ Horizontal-Ellipsis ] is the integer part) corresponding to polarized phases with ruptures singlet pairs. A nonmonotonic behavior observed for the magnetic susceptibility of an easy-plane cluster is typical of gap magnets. The spin gap between the ground state and excited states is proportional to the anisotropy parameter.

  19. Internal magnetic field measurement on C-2 field-reversed configuration plasmas.

    PubMed

    Gota, H; Thompson, M C; Knapp, K; Van Drie, A D; Deng, B H; Mendoza, R; Guo, H Y; Tuszewski, M

    2012-10-01

    A long-lived field-reversed configuration (FRC) plasma has been produced in the C-2 device by dynamically colliding and merging two oppositely directed, highly supersonic compact toroids (CTs). The reversed-field structure of the translated CTs and final merged-FRC state have been directly verified by probing the internal magnetic field structure using a multi-channel magnetic probe array near the midplane of the C-2 confinement chamber. Each of the two translated CTs exhibits significant toroidal fields (B(t)) with opposite helicity, and a relatively large B(t) remains inside the separatrix after merging.

  20. Magnetization reversal phenomena in (Cr0.70Ti0.30)5S6

    NASA Astrophysics Data System (ADS)

    Hashimoto, Satoshi; Matsuda, Yuji; Sato, Tetsuya; Anzai, Shuichiro

    2005-12-01

    Magnetization reversal phenomena (MRP) along magnetic order-order transitions have recently been reported on impurity-doped magnetic systems. Because imperfect long-range magnetic order exists in these systems, it is expected that a systematic investigation of MRP will give physical information on thermomagnetic processes of magnetic systems in the range from the micro- to nanoscales. As a typical order-order transition (a state doubly modulated by helical and canting orders to a collinear ferrimagnetic state) has been known to occur on Cr5S6 at a transition temperature Tt, we investigate the magnetizations of (Cr0.70Ti0.30)5S6 on heating and cooling runs in various magnetic fields. At 20Oe, the field-cooled magnetization just below the Curie temperature has a positive sign; the sign turns negative below the compensation temperature TCM (first step) and finally returns to positive below Tt (second step). The first-step MRP observed in this system is explained by the potential barriers resulting from anisotropy energy when the preferred direction of collinear ferrimagnetic moment reverses. The proposed mechanism for second-step MRP is the pinning effect caused by the impurity atoms (Ti) in the helical long-range-order chains. Comparing other examples of MRPs, we discuss the roles of local impurity centers in the thermomagnetic process in magnetic order-order transitions.

  1. Buffer layer annealing effects on the magnetization reversal process in Pd/Co/Pd systems

    NASA Astrophysics Data System (ADS)

    Fassatoui, A.; Belhi, R.; Vogel, J.; Abdelmoula, K.

    2016-12-01

    We have investigated the effect of annealing the buffer layer on the magnetization reversal behavior in Pd/Co/Pd thin films using magneto-optical Kerr microscopy. It was found that annealing the buffer layer at 150 °C for 1 h decreases the coercivity and increases the saturation magnetization and the effective magnetic anisotropy constant. This study also shows that the annealing induces a change of the magnetization reversal from a mixed nucleation and domain wall propagation process to one dominated by domain wall propagation. This result demonstrates that the main effect of annealing the buffer layer is to decrease the domain wall pinning in the Co layer, favoring the domain wall propagation mode.

  2. Linear and nonlinear magnetic properties of ferrofluids

    NASA Astrophysics Data System (ADS)

    Szalai, I.; Nagy, S.; Dietrich, S.

    2015-10-01

    Within a high-magnetic-field approximation, employing Ruelle's algebraic perturbation theory, a field-dependent free-energy expression is proposed which allows one to determine the magnetic properties of ferrofluids modeled as dipolar hard-sphere systems. We compare the ensuing magnetization curves, following from this free energy, with those obtained by Ivanov and Kuznetsova [Phys. Rev. E 64, 041405 (2001), 10.1103/PhysRevE.64.041405] as well as with new corresponding Monte Carlo simulation data. Based on the power-series expansion of the magnetization, a closed expression for the magnetization is also proposed, which is a high-density extension of the corresponding equation of Ivanov and Kuznetsova. From both magnetization equations the zero-field susceptibility expression due to Tani et al. [Mol. Phys. 48, 863 (1983), 10.1080/00268978300100621] can be obtained, which is in good agreement with our MC simulation results. From the closed expression for the magnetization the second-order nonlinear magnetic susceptibility is also derived, which shows fair agreement with the corresponding MC simulation data.

  3. Linear and nonlinear magnetic properties of ferrofluids.

    PubMed

    Szalai, I; Nagy, S; Dietrich, S

    2015-10-01

    Within a high-magnetic-field approximation, employing Ruelle's algebraic perturbation theory, a field-dependent free-energy expression is proposed which allows one to determine the magnetic properties of ferrofluids modeled as dipolar hard-sphere systems. We compare the ensuing magnetization curves, following from this free energy, with those obtained by Ivanov and Kuznetsova [Phys. Rev. E 64, 041405 (2001)] as well as with new corresponding Monte Carlo simulation data. Based on the power-series expansion of the magnetization, a closed expression for the magnetization is also proposed, which is a high-density extension of the corresponding equation of Ivanov and Kuznetsova. From both magnetization equations the zero-field susceptibility expression due to Tani et al. [Mol. Phys. 48, 863 (1983)] can be obtained, which is in good agreement with our MC simulation results. From the closed expression for the magnetization the second-order nonlinear magnetic susceptibility is also derived, which shows fair agreement with the corresponding MC simulation data. PMID:26565247

  4. Graphene as a reversible spin manipulator of molecular magnets.

    PubMed

    Bhandary, Sumanta; Ghosh, Saurabh; Herper, Heike; Wende, Heiko; Eriksson, Olle; Sanyal, Biplab

    2011-12-16

    One of the primary objectives in molecular nanospintronics is to manipulate the spin states of organic molecules with a d-electron center, by suitable external means. In this Letter, we demonstrate by first principles density functional calculations, as well as second order perturbation theory, that a strain induced change of the spin state, from S=1→S=2, takes place for an iron porphyrin (FeP) molecule deposited at a divacancy site in a graphene lattice. The process is reversible in the sense that the application of tensile or compressive strains in the graphene lattice can stabilize FeP in different spin states, each with a unique saturation moment and easy axis orientation. The effect is brought about by a change in Fe-N bond length in FeP, which influences the molecular level diagram as well as the interaction between the C atoms of the graphene layer and the molecular orbitals of FeP.

  5. Graphene as a Reversible Spin Manipulator of Molecular Magnets

    NASA Astrophysics Data System (ADS)

    Bhandary, Sumanta; Ghosh, Saurabh; Herper, Heike; Wende, Heiko; Eriksson, Olle; Sanyal, Biplab

    2011-12-01

    One of the primary objectives in molecular nanospintronics is to manipulate the spin states of organic molecules with a d-electron center, by suitable external means. In this Letter, we demonstrate by first principles density functional calculations, as well as second order perturbation theory, that a strain induced change of the spin state, from S=1→S=2, takes place for an iron porphyrin (FeP) molecule deposited at a divacancy site in a graphene lattice. The process is reversible in the sense that the application of tensile or compressive strains in the graphene lattice can stabilize FeP in different spin states, each with a unique saturation moment and easy axis orientation. The effect is brought about by a change in Fe-N bond length in FeP, which influences the molecular level diagram as well as the interaction between the C atoms of the graphene layer and the molecular orbitals of FeP.

  6. Reversals.

    ERIC Educational Resources Information Center

    National Center on Educational Media and Materials for the Handicapped, Columbus, OH.

    Selected from the National Instructional Materials Information System (NIMIS)--a computer based on-line interactive retrieval system on special education materials--the bibliography covers nine materials for remediating reversals in handicapped students at the early childhood and elementary levels. Entries are presented in order of NIMIS accession…

  7. Magnetic properties and energy-mapping analysis.

    PubMed

    Xiang, Hongjun; Lee, Changhoon; Koo, Hyun-Joo; Gong, Xingao; Whangbo, Myung-Hwan

    2013-01-28

    The magnetic energy levels of a given magnetic solid are closely packed in energy because the interactions between magnetic ions are weak. Thus, in describing its magnetic properties, one needs to generate its magnetic energy spectrum by employing an appropriate spin Hamiltonian. In this review article we discuss how to determine and specify a necessary spin Hamiltonian in terms of first principles electronic structure calculations on the basis of energy-mapping analysis and briefly survey important concepts and phenomena that one encounters in reading the current literature on magnetic solids. Our discussion is given on a qualitative level from the perspective of magnetic energy levels and electronic structures. The spin Hamiltonian appropriate for a magnetic system should be based on its spin lattice, i.e., the repeat pattern of its strong magnetic bonds (strong spin exchange paths), which requires one to evaluate its Heisenberg spin exchanges on the basis of energy-mapping analysis. Other weaker energy terms such as Dzyaloshinskii-Moriya (DM) spin exchange and magnetocrystalline anisotropy energies, which a spin Hamiltonian must include in certain cases, can also be evaluated by performing energy-mapping analysis. We show that the spin orientation of a transition-metal magnetic ion can be easily explained by considering its split d-block levels as unperturbed states with the spin-orbit coupling (SOC) as perturbation, that the DM exchange between adjacent spin sites can become comparable in strength to the Heisenberg spin exchange when the two spin sites are not chemically equivalent, and that the DM interaction between rare-earth and transition-metal cations is governed largely by the magnetic orbitals of the rare-earth cation. PMID:23128376

  8. Properties and biomedical applications of magnetic nanoparticles

    NASA Astrophysics Data System (ADS)

    Regmi, Rajesh Kumar

    Magnetic nanoparticles have a number of unique properties, making them promising agents for applications in medicine including magnetically targeted drug delivery, magnetic hyperthermia, magnetic resonance imaging, and radiation therapy. They are biocompatible and can also be coated with biocompatible surfactants, which may be further functionalized with optically and therapeutically active molecules. These nanoparticles can be manipulated with non-invasive external magnetic field to produce heat, target specific site, and monitor their distribution in vivo. Within this framework, we have investigated a number of biomedical applications of these nanoparticles. We synthesized a thermosensitive microgel with iron oxide adsorbed on its surface. An alternating magnetic field applied to these nanocomposites heated the system and triggered the release of an anticancer drug mitoxantrone. We also parameterized the chain length dependence of drug release from dextran coated iron oxide nanoparticles, finding that both the release rate and equilibrium release fraction depend on the molecular mass of the surfactant. Finally, we also localized dextran coated iron oxide nanoparticles labeled with tat peptide to the cell nucleus, which permits this system to be used for a variety of biomedical applications. Beyond investigating magnetic nanoparticles for biomedical applications, we also studied their magnetohydrodynamic and dielectric properties in solution. Magnetohydrodynamic properties of ferrofluid can be controlled by appropriate selection of surfactant and deielctric measurement showed magnetodielectric coupling in this system. We also established that some complex low temperature spin structures are suppressed in Mn3O4 nanoparticles, which has important implications for nanomagnetic devices. Furthermore, we explored exchange bias effects in Ni-NiO core-shell nanoparticles. Finally, we also performed extensive magnetic studies in nickel metalhydride (NiMH) batteries to

  9. (The relationship between microstructure and magnetic properties in high-energy permanent magnets characterized by polytwinned structures)

    SciTech Connect

    Not Available

    1992-01-01

    This report summarizes the results of a study of the relationship between microstructure and magnetic properties in a unique genre of ferromagnetic material characterized by a polysynthetically twinned structure which arises during solid state transformation. These results stem from the work over a period of approximately 27 months of a nominal 3 year grant period. The report also contains a proposal to extend the research project for an additional 3 years. The polytwinned structures produce an inhomogeneous magnetic medium in which the easy axis of magnetization varies quasi-periodically giving rise to special domain configurations which are expected to markedly influence the mechanism of magnetization reversal and hysteresis behavior of these materials in bulk or thin films. The extraordinary permanent magnet properties exhibited by the well-known Co-Pt alloys as well as the Fe-Pt and Fe-Pd systems near the equiatomic composition derive from the formation of a polytwinned microstructure.

  10. [The relationship between microstructure and magnetic properties in high-energy permanent magnets characterized by polytwinned structures

    SciTech Connect

    Not Available

    1992-07-01

    This report summarizes the results of a study of the relationship between microstructure and magnetic properties in a unique genre of ferromagnetic material characterized by a polysynthetically twinned structure which arises during solid state transformation. These results stem from the work over a period of approximately 27 months of a nominal 3 year grant period. The report also contains a proposal to extend the research project for an additional 3 years. The polytwinned structures produce an inhomogeneous magnetic medium in which the easy axis of magnetization varies quasi-periodically giving rise to special domain configurations which are expected to markedly influence the mechanism of magnetization reversal and hysteresis behavior of these materials in bulk or thin films. The extraordinary permanent magnet properties exhibited by the well-known Co-Pt alloys as well as the Fe-Pt and Fe-Pd systems near the equiatomic composition derive from the formation of a polytwinned microstructure.

  11. Multifunctional hybrid nanocomposites with magnetically controlled reversible shape-memory effect.

    PubMed

    Razzaq, Muhammad Yasar; Behl, Marc; Kratz, Karl; Lendlein, Andreas

    2013-10-25

    Magneto-sensitivity and a thermo-sensitive reversible shape-memory effect have been successfully integrated into a hybrid nanocomposite, resulting in a magnetically controlled actuator. The complex requirements for gaining this multifunctionality are fulfilled by combining netpoints on the molecular and nano level in a polyesterurethane network prepared from hydroxyl group decorated magnetic nanoparticles, crystallizable star-shaped poly(ω-pentadecalactone) precursors, and a diisocyanate.

  12. Burnt clay magnetic properties and palaeointensity determination

    NASA Astrophysics Data System (ADS)

    Avramova, Mariya; Lesigyarski, Deyan

    2014-05-01

    Burnt clay structures found in situ are the most valuable materials for archaeomagnetic studies. From these materials the full geomagnetic field vector described by inclination, declination and intensity can be retrieved. The reliability of the obtained directional results is related to the precision of samples orientation and the accuracy of characteristic remanence determination. Palaeointensity evaluations depend on much more complex factors - stability of carried remanent magnetization, grain-size distribution of magnetic particles and mineralogical transformations during heating. In the last decades many efforts have been made to shed light over the reasons for the bad success rate of palaeointensity experiments. Nevertheless, sometimes the explanation of the bad archaeointensity results with the magnetic properties of the studied materials is quite unsatisfactory. In order to show how difficult is to apply a priory strict criteria for the suitability of a given collection of archaeomagnetic materials, artificial samples formed from four different baked clays are examined. Two of the examined clay types were taken from clay deposits from different parts of Bulgaria and two clays were taken from ancient archaeological baked clay structures from the Central part of Bulgaria and the Black sea coast, respectively. The samples formed from these clays were repeatedly heated in known magnetic field to 700oC. Different analyses were performed to obtain information about the mineralogical content and magnetic properties of the samples. The obtained results point that all clays reached stable magnetic mineralogy after the repeated heating to 700oC, the main magnetic mineral is of titano/magnetite type and the magnetic particles are predominantly with pseudo single domain grain sizes. In spite that, the magnetic properies of the studied clays seem to be very similar, reliable palaeointensity results were obtained only from the clays coming from clay deposits. The

  13. Determination of the anisotropies and reversal process in exchange-bias bilayers using a rotational magnetization curve approach

    SciTech Connect

    Sui Wenbo; Zhu Jingyi; Li Jinyun; Chai Guozhi; Jiang Changjun; Fan Xiaolong; Xue Desheng

    2011-05-15

    Rotational magnetization curves of the exchange-bias bilayers were investigated based on the Stoner-Wohlfarth model, which can be grouped into three cases according to the magnetization reversal process. The unidirectional anisotropic field H{sub E} = 41.4 Oe, the uniaxial anisotropic field H{sub k} = 4.2 Oe and the accurate direction of the easy axis of our FeNi/FeMn exchange-bias bilayers were obtained by fitting their experimental rotational magnetization curves. During the rotational process the magnetization reversal of the bilayers is a coherent rotation with a critical magnetization reversal field H{sub 1} = 41.372 Oe.

  14. Cryogenic properties of dispersion strengthened copper for high magnetic fields

    NASA Astrophysics Data System (ADS)

    Toplosky, V. J.; Han, K.; Walsh, R. P.; Swenson, C. A.

    2014-01-01

    Cold deformed copper matrix composite conductors, developed for use in the 100 tesla multi-shot pulsed magnet at the National High Magnetic Field Laboratory (NHMFL), have been characterized. The conductors are alumina strengthened copper which is fabricated by cold drawing that introduces high dislocation densities and high internal stresses. Both alumina particles and high density of dislocations provide us with high tensile strength and fatigue endurance. The conductors also have high electrical conductivities because alumina has limited solubility in Cu and dislocations have little scattering effect on conduction electrons. Such a combination of high strength and high conductivity makes it an excellent candidate over other resistive magnet materials. Thus, characterization is carried out by tensile testing and fully reversible fatigue testing. In tensile tests, the material exceeds the design criteria parameters. In the fatigue tests, both the load and displacement were measured and used to control the amplitude of the tests to simulate the various loading conditions in the pulsed magnet which is operated at 77 K in a non-destructive mode. In order to properly simulate the pulsed magnet operation, strain-controlled tests were more suitable than load controlled tests. For the dispersion strengthened coppers, the strengthening mechanism of the aluminum oxide provided better tensile and fatigue properties over convention copper.

  15. Cryogenic properties of dispersion strengthened copper for high magnetic fields

    SciTech Connect

    Toplosky, V. J.; Han, K.; Walsh, R. P.; Swenson, C. A.

    2014-01-27

    Cold deformed copper matrix composite conductors, developed for use in the 100 tesla multi-shot pulsed magnet at the National High Magnetic Field Laboratory (NHMFL), have been characterized. The conductors are alumina strengthened copper which is fabricated by cold drawing that introduces high dislocation densities and high internal stresses. Both alumina particles and high density of dislocations provide us with high tensile strength and fatigue endurance. The conductors also have high electrical conductivities because alumina has limited solubility in Cu and dislocations have little scattering effect on conduction electrons. Such a combination of high strength and high conductivity makes it an excellent candidate over other resistive magnet materials. Thus, characterization is carried out by tensile testing and fully reversible fatigue testing. In tensile tests, the material exceeds the design criteria parameters. In the fatigue tests, both the load and displacement were measured and used to control the amplitude of the tests to simulate the various loading conditions in the pulsed magnet which is operated at 77 K in a non-destructive mode. In order to properly simulate the pulsed magnet operation, strain-controlled tests were more suitable than load controlled tests. For the dispersion strengthened coppers, the strengthening mechanism of the aluminum oxide provided better tensile and fatigue properties over convention copper.

  16. Light-induced magnetization reversal of high-anisotropy TbCo alloy films

    NASA Astrophysics Data System (ADS)

    Alebrand, Sabine; Gottwald, Matthias; Hehn, Michel; Steil, Daniel; Cinchetti, Mirko; Lacour, Daniel; Fullerton, Eric E.; Aeschlimann, Martin; Mangin, Stéphane

    2012-10-01

    Magnetization reversal using circularly polarized light provides a way to control magnetization without any external magnetic field and has the potential to revolutionize magnetic data storage. However, in order to reach ultra-high density data storage, high anisotropy media providing thermal stability are needed. Here, we evidence all-optical magnetization switching for different TbxCo1-x ferrimagnetic alloy compositions using fs- and ps-laser pulses and demonstrate all-optical switching for films with anisotropy fields reaching 6 T corresponding to anisotropy constants of 3 × 106 ergs/cm3. Optical magnetization switching is observed only for alloy compositions where the compensation temperature can be reached through sample heating.

  17. Magnetic Properties of 3D Printed Toroids

    NASA Astrophysics Data System (ADS)

    Bollig, Lindsey; Otto, Austin; Hilpisch, Peter; Mowry, Greg; Nelson-Cheeseman, Brittany; Renewable Energy; Alternatives Lab (REAL) Team

    Transformers are ubiquitous in electronics today. Although toroidal geometries perform most efficiently, transformers are traditionally made with rectangular cross-sections due to the lower manufacturing costs. Additive manufacturing techniques (3D printing) can easily achieve toroidal geometries by building up a part through a series of 2D layers. To get strong magnetic properties in a 3D printed transformer, a composite filament is used containing Fe dispersed in a polymer matrix. How the resulting 3D printed toroid responds to a magnetic field depends on two structural factors of the printed 2D layers: fill factor (planar density) and fill pattern. In this work, we investigate how the fill factor and fill pattern affect the magnetic properties of 3D printed toroids. The magnetic properties of the printed toroids are measured by a custom circuit that produces a hysteresis loop for each toroid. Toroids with various fill factors and fill patterns are compared to determine how these two factors can affect the magnetic field the toroid can produce. These 3D printed toroids can be used for numerous applications in order to increase the efficiency of transformers by making it possible for manufacturers to make a toroidal geometry.

  18. Refocusing properties of periodic magnetic fields

    NASA Technical Reports Server (NTRS)

    Stankiewicz, N.

    1976-01-01

    The use of depressed collectors for the efficient collection of spent beams from linear-beam microwave tubes depends on a refocusing procedure in which the space charge forces and transverse velocity components are reduced. The refocusing properties are evaluated of permanent magnet configurations whose axial fields are approximated by constant plateaus or linearly varying fields. The results provide design criteria and show that the refocusing properties can be determined from the plateau fields alone.

  19. First order reversal curve investigation of the hard and soft magnetic phases of annealed CoFeCu nanowire arrays

    NASA Astrophysics Data System (ADS)

    Almasi-Kashi, M.; Ramazani, A.; Golafshan, E.; Arefpour, M.; Jafari-Khamse, E.

    2013-11-01

    (CoFe)1-xCux (x=0.12-0.84) nanowire arrays were ac-pulse electrodeposited into anodic aluminum oxide templates. The electrodeposition was performed in a constant electrolyte while Cu content was controlled by off-time between pulses. Nanowires with 30 nm diameter and the certain lengths with the both bcc-CoFe and fcc-Cu phases were obtained. Magnetization and coercivity of the nanowires decreased with increasing the Cu content. Annealing improved the coercivity and a remarkable increase in magnetization of nanowires with high Cu contents was observed. A two-phase treatment was seen for annealed samples with high Cu contents. First order reversal curves showed a hard magnetic phase with almost constant magnetic properties and coercivity of ~2500 Oe. The results showed that main source of the various magnetic behaviors of the samples may be attributed to increase in soft magnetic phase. A single domain treatment with a narrow interacting field and coercive field distributions was also observed for the annealed samples with high Cu content.

  20. Magnetic design calculation and FRC formation modeling for the field reversed experiment liner

    SciTech Connect

    Dorf, L. A.; Intrator, T. P.; Renneke, R.; Hsu, S. C.; Wurden, G. A.; Awe, T.; Siemon, R.; Semenov, V. E.

    2008-10-01

    Integrated magnetic modeling and design are important to meet the requirements for (1) formation, (2) translation, and (3) compression of a field reversed configuration (FRC) for magnetized target fusion. Off-the-shelf solutions do not exist for many generic design issues. A predictive capability for time-dependent magnetic diffusion in realistically complicated geometry is essential in designing the experiment. An eddy-current code was developed and used to compute the mutual inductances between driven magnetic coils and passive magnetic shields (flux excluder plates) to calculate the self-consistent axisymmetric magnetic fields during the first two stages. The plasma in the formation stage was modeled as an immobile solid cylinder with selectable constant resistivity and magnetic flux that was free to readjust itself. It was concluded that (1) use of experimentally obtained anomalously large plasma resistivity in magnetic diffusion simulations is sufficient to predict magnetic reconnection and FRC formation, (2) comparison of predicted and experimentally observed timescales for FRC Ohmic decay shows good agreement, and (3) for the typical range of resistivities, the magnetic null radius decay rate scales linearly with resistivity. The last result can be used to predict the rate of change in magnetic flux outside of the separatrix (equal to the back-emf loop voltage), and thus estimate a minimum {theta}-coil loop voltage required to form an FRC.

  1. Magnetic properties of the Imilac Pallasite

    NASA Astrophysics Data System (ADS)

    Hopkins, J.; Tarduno, J. A.; Cottrell, R. D.

    2009-12-01

    Pallasites are a type of stony-iron meteorite containing olivine crystals within an iron-nickel alloy. Magnetic inclusions, which can be found in the olivine crystals, may contain a memory of exposure to ancient magnetic fields. By studying the properties of the magnetic inclusions, we can learn more about the fields present during formation and how this relates to the evolution of the parent bodies. An important step in this research is to find appropriate samples to measure. The best magnetic recorders are single domain (SD) magnetic grains; to search for potential carriers of SD grains we separated gem-like olivine crystals from a sample of the Imilac pallasite. Crystal fragments were cleaned to remove iron staining; the fragments were further scanned with a visible light microscope to exclude samples with large (potentially multidomain) magnetic inclusions. Measurements of these select samples with an Alternating Gradient Force Magnetometer (AGFM) suggest the presence of single domain magnetic inclusions suitable for the preservation of paleofields. We will present preliminary paleointensity analyses of these samples. This is a presentation of results collected during a REU summer program at the University of Rochester.

  2. Magnetic dipole discharges. I. Basic properties

    SciTech Connect

    Stenzel, R. L.; Urrutia, J. M.; Teodorescu-Soare, C. T.; Ionita, C.; Schrittwieser, R.

    2013-08-15

    A simple discharge is described which uses a permanent magnet as a cold cathode and the metallic chamber wall as an anode. The magnet's equator is biased strongly negative, which produces secondary electrons due to the impact of energetic ions. The emitted electrons are highly confined by the strong dipolar magnetic field and the negative potential in the equatorial plane of the magnet. The emitted electrons ionize near the sheath and produce further electrons, which drift across field lines to the anode while the nearly unmagnetized ions are accelerated back to the magnet. A steady state discharge is maintained at neutral pressures above 10{sup −3} mbar. This is the principle of magnetron discharges, which commonly use cylindrical and planar cathodes rather than magnetic dipoles as cathodes. The discharge properties have been investigated in steady state and pulsed mode. Different magnets and geometries have been employed. The role of a background plasma has been investigated. Various types of instabilities have been observed such as sheath oscillations, current-driven turbulence, relaxation instabilities due to ionization, and high frequency oscillations created by sputtering impulses, which are described in more detail in companion papers. The discharge has also been operated in reactive gases and shown to be useful for sputtering applications.

  3. Magnetic properties of metal-substituted haematite

    NASA Astrophysics Data System (ADS)

    Wells, M. A.; Fitzpatrick, R. W.; Gilkes, R. J.; Dobson, J.

    1999-08-01

    Mineral and isothermal magnetic properties of Al-, Mn- and Ni-substituted haematites were characterized and their relationships evaluated in order to interpret better the results of magnetic analyses of soils and recent sediments. Aluminium, manganese and nickel haematites generally behaved as single-domain (SD) particles. The influence of incorporated Al on the magnetic behaviour of haematite was consistent with Al acting as a paramagnetic dilutent. Mass magnetic susceptibility (chi) and SIRM_800 decreased as the level of Al substitution increased. Incorporation of Mn and Ni increased chi, which could be associated with enhancement of the spin canting effect of haematite. The stability of SIRM_800 to demagnetization for Al-haematite appears to be related to a defect mechanism associated with the development of smaller crystallites arising from Al substitution. Magnetic domain rotation or flipping was probably inhibited, being blocked by structural defects during magnetization and demagnetization, and resulted in a low but stable partial SIRM (SIRM_800). %IRM/SIRM_800 demagnetization curves and estimated (B_o)_CR values of <=100 mT for Mn-haematite indicate pseudo-single-domain/multidomain-like behaviour despite Mn-haematite having particle and crystallite dimensions similar to Ni-haematite, which did not show this behaviour. Data indicate that parameters involving unsaturated, partial SIRM should be used with caution in magnetic studies of soils and sediments.

  4. Time-reversal symmetry breaking and spontaneous Hall effect without magnetic dipole order.

    PubMed

    Machida, Yo; Nakatsuji, Satoru; Onoda, Shigeki; Tayama, Takashi; Sakakibara, Toshiro

    2010-01-14

    Spin liquids are magnetically frustrated systems, in which spins are prevented from ordering or freezing, owing to quantum or thermal fluctuations among degenerate states induced by the frustration. Chiral spin liquids are a hypothetical class of spin liquids in which the time-reversal symmetry is macroscopically broken in the absence of an applied magnetic field or any magnetic dipole long-range order. Even though such chiral spin-liquid states were proposed more than two decades ago, an experimental realization and observation of such states has remained a challenge. One of the characteristic order parameters in such systems is a macroscopic average of the scalar spin chirality, a solid angle subtended by three nearby spins. In previous experimental reports, however, the spin chirality was only parasitic to the non-coplanar spin structure associated with a magnetic dipole long-range order or induced by the applied magnetic field, and thus the chiral spin-liquid state has never been found. Here, we report empirical evidence that the time-reversal symmetry can be broken spontaneously on a macroscopic scale in the absence of magnetic dipole long-range order. In particular, we employ the anomalous Hall effect to directly probe the broken time-reversal symmetry for the metallic frustrated magnet Pr(2)Ir(2)O(7). An onset of the Hall effect is observed at zero field in the absence of uniform magnetization, within the experimental accuracy, suggesting an emergence of a chiral spin liquid. The origin of this spontaneous Hall effect is ascribed to chiral spin textures, which are inferred from the magnetic measurements indicating the spin ice-rule formation. PMID:20010605

  5. ON POLAR MAGNETIC FIELD REVERSAL AND SURFACE FLUX TRANSPORT DURING SOLAR CYCLE 24

    SciTech Connect

    Sun, Xudong; Todd Hoeksema, J.; Liu, Yang; Zhao, Junwei

    2015-01-10

    As each solar cycle progresses, remnant magnetic flux from active regions (ARs) migrates poleward to cancel the old-cycle polar field. We describe this polarity reversal process during Cycle 24 using four years (2010.33-2014.33) of line-of-sight magnetic field measurements from the Helioseismic and Magnetic Imager. The total flux associated with ARs reached maximum in the north in 2011, more than two years earlier than the south; the maximum is significantly weaker than Cycle 23. The process of polar field reversal is relatively slow, north-south asymmetric, and episodic. We estimate that the global axial dipole changed sign in 2013 October; the northern and southern polar fields (mean above 60° latitude) reversed in 2012 November and 2014 March, respectively, about 16 months apart. Notably, the poleward surges of flux in each hemisphere alternated in polarity, giving rise to multiple reversals in the north. We show that the surges of the trailing sunspot polarity tend to correspond to normal mean AR tilt, higher total AR flux, or slower mid-latitude near-surface meridional flow, while exceptions occur during low magnetic activity. In particular, the AR flux and the mid-latitude poleward flow speed exhibit a clear anti-correlation. We discuss how these features can be explained in a surface flux transport process that includes a field-dependent converging flow toward the ARs, a characteristic that may contribute to solar cycle variability.

  6. Ultra-fast magnetic vortex core reversal by a local field pulse

    SciTech Connect

    Rückriem, R.; Albrecht, M.; Schrefl, T.

    2014-02-03

    Magnetic vortex core reversal of a 20-nm-thick permalloy disk with a diameter of 100 nm was studied by micromagnetic simulations. By applying a global out-of-plane magnetic field pulse, it turned out that the final core polarity is very sensitive to pulse width and amplitude, which makes it hard to control. The reason for this phenomenon is the excitation of radial spin waves, which dominate the reversal process. The excitation of spin waves can be strongly suppressed by applying a local field pulse within a small area at the core center. With this approach, ultra-short reversal times of about 15 ps were achieved, which are ten times faster compared to a global pulse.

  7. Hysteretic magnetic pinning and reversible resistance switching in high-temperature superconductor/ferromagnet multilayers

    NASA Astrophysics Data System (ADS)

    Visani, C.; Metaxas, P. J.; Collaudin, A.; Calvet, B.; Bernard, R.; Briatico, J.; Deranlot, C.; Bouzehouane, K.; Villegas, J. E.

    2011-08-01

    We study a high-critical temperature superconducting (YBa2Cu3O7-δ)/ferromagnetic (Co/Pt multilayer) hybrid that exhibits resistance switching driven by the magnetic history: depending on the direction of the external field, a pronounced decrease or increase of the mixed-state resistance is observed as magnetization reversal occurs within the Co/Pt multilayer. We demonstrate that stray magnetic fields cause these effects via (i) creation of vortices/antivortices and (ii) magnetostatic pinning of vortices that are induced by the external field.

  8. An Enhanced Nonlinear Critical Gradient for Electron Turbulent Transport due to Reversed Magnetic Shear

    SciTech Connect

    Peterson, J. L.; Hammet, G. W.; Mikkelsen, D. R.; Yuh, H. Y.; Candy, J.; Guttenfelder, W.; Kaye, S. M.; LeBlanc, B.

    2011-05-11

    The first nonlinear gyrokinetic simulations of electron internal transport barriers (e-ITBs) in the National Spherical Torus Experiment show that reversed magnetic shear can suppress thermal transport by increasing the nonlinear critical gradient for electron-temperature-gradient-driven turbulence to three times its linear critical value. An interesting feature of this turbulence is non- linearly driven off-midplane radial streamers. This work reinforces the experimental observation that magnetic shear is likely an effective way of triggering and sustaining e-ITBs in magnetic fusion devices.

  9. Numerical analysis of thermally assisted spin-transfer torque magnetization reversal in synthetic ferrimagnetic free layers

    SciTech Connect

    Shen, J.; Shi, M.; Tanaka, T. Matsuyama, K.

    2015-05-07

    The spin transfer torque magnetization reversal of synthetic ferrimagnetic free layers under pulsed temperature rise was numerically studied by solving the Landau–Lifshitz–Gilbert equation, taking into account the stochastic random fields, the temperature dependence of magnetic parameters, and the spin torque terms. The anti-parallel magnetization configuration was retained at the elevated temperature, due to interlayer dipole coupling. A significant thermal assistance effect, resulting in a 40% reduction in the switching current, was demonstrated during a nanosecond pulsed temperature rise up to 77% of the Curie temperature.

  10. Influence of shape, size and internal structure on magnetic properties of core-edge nanodots with perpendicular anisotropy

    SciTech Connect

    Milińska, E. Wawro, A.

    2014-11-21

    The properties of perpendicularly magnetized isolated nanodots different in shape, size, and internal structure are simulated by micromagnetic calculations. Investigated dots are magnetically uniform, or they are composed of a core and an edge characterized by different anisotropy—stronger or weaker than that of the core. Based on calculated hysteresis loops, we discuss in details the magnetization reversal processes, stability of magnetic structures, and spin configurations in the dots.

  11. Field-free magnetization reversal by spin-Hall effect and exchange bias

    NASA Astrophysics Data System (ADS)

    van den Brink, A.; Vermijs, G.; Solignac, A.; Koo, J.; Kohlhepp, J. T.; Swagten, H. J. M.; Koopmans, B.

    2016-03-01

    As the first magnetic random access memories are finding their way onto the market, an important issue remains to be solved: the current density required to write magnetic bits becomes prohibitively high as bit dimensions are reduced. Recently, spin-orbit torques and the spin-Hall effect in particular have attracted significant interest, as they enable magnetization reversal without high current densities running through the tunnel barrier. For perpendicularly magnetized layers, however, the technological implementation of the spin-Hall effect is hampered by the necessity of an in-plane magnetic field for deterministic switching. Here we interface a thin ferromagnetic layer with an anti-ferromagnetic material. An in-plane exchange bias is created and shown to enable field-free S HE-driven magnetization reversal of a perpendicularly magnetized Pt/Co/IrMn structure. Aside from the potential technological implications, our experiment provides additional insight into the local spin structure at the ferromagnetic/anti-ferromagnetic interface.

  12. Field-free magnetization reversal by spin-Hall effect and exchange bias.

    PubMed

    van den Brink, A; Vermijs, G; Solignac, A; Koo, J; Kohlhepp, J T; Swagten, H J M; Koopmans, B

    2016-01-01

    As the first magnetic random access memories are finding their way onto the market, an important issue remains to be solved: the current density required to write magnetic bits becomes prohibitively high as bit dimensions are reduced. Recently, spin-orbit torques and the spin-Hall effect in particular have attracted significant interest, as they enable magnetization reversal without high current densities running through the tunnel barrier. For perpendicularly magnetized layers, however, the technological implementation of the spin-Hall effect is hampered by the necessity of an in-plane magnetic field for deterministic switching. Here we interface a thin ferromagnetic layer with an anti-ferromagnetic material. An in-plane exchange bias is created and shown to enable field-free S HE-driven magnetization reversal of a perpendicularly magnetized Pt/Co/IrMn structure. Aside from the potential technological implications, our experiment provides additional insight into the local spin structure at the ferromagnetic/anti-ferromagnetic interface. PMID:26940861

  13. Dynamic in situ observation of voltage-driven repeatable magnetization reversal at room temperature.

    PubMed

    Gao, Ya; Hu, Jia-Mian; Nelson, C T; Yang, T N; Shen, Y; Chen, L Q; Ramesh, R; Nan, C W

    2016-03-31

    Purely voltage-driven, repeatable magnetization reversal provides a tantalizing potential for the development of spintronic devices with a minimum amount of power consumption. Substantial progress has been made in this subject especially on magnetic/ferroelectric heterostructures. Here, we report the in situ observation of such phenomenon in a NiFe thin film grown directly on a rhombohedral Pb(Mg1/3Nb2/3)0.7Ti0.3O3(PMN-PT) ferroelectric crystal. Under a cyclic voltage applied perpendicular to the PMN-PT without a magnetic field, the local magnetization of NiFe can be repetitively reversed through an out-of-plane excursion and then back into the plane. Using phase field simulations we interpret magnetization reversal as a synergistic effect of the metastable ferroelastic switching in the PMN-PT and an electrically rotatable local exchange bias field arising from the heterogeneously distributed NiO clusters at the interface.

  14. Magnetization reversal in asymmetric trilayer dots: effect of the interlayer magnetostatic coupling

    PubMed Central

    2014-01-01

    The spin structure and magnetization reversal in Co/insulator/Fe trilayer nanodots are investigated by micromagnetic simulations. The vortex and C-state are found and the magnetization reversal is dominated by the shape asymmetry of the dots, which is produced by cutting off a fraction of the circular dot. The vortex chirality is thus controlled by the magnetic field direction. On the other hand, the magnetostatic interaction between the top and bottom magnetic layers has interesting influence on the dot reversal process, where the magnetocrystalline anisotropy direction of the Co layer is allowed to vary within the layer plane. The combined effect of these two aspects is discussed on the base of dot coercivity, remanent magnetization, vortex nucleation and annihilation, and the bias of the Fe layer hysteresis loop. While leading to a new S-state in circle dots, the interlayer interaction facilitates the formation of C-state in asymmetric dots, which reduces the vortex nucleation field. The bias effect of all dots is decreased with the deviation of the Co layer easy axis from the field direction. Unlike the circle and semicircle dots, the field range of the vortex state in other asymmetric dots increases with the angle between the cutting direction and the Co layer anisotropy. Additionally, vortex ranges in less asymmetric dots even larger than that in the circle dots are evidenced unexpectedly. Therefore, the control of the vortex chirality and enhancement of the vortex range are found simultaneously. PMID:24589295

  15. Dynamic in situ observation of voltage-driven repeatable magnetization reversal at room temperature

    NASA Astrophysics Data System (ADS)

    Gao, Ya; Hu, Jia-Mian; Nelson, C. T.; Yang, T. N.; Shen, Y.; Chen, L. Q.; Ramesh, R.; Nan, C. W.

    2016-03-01

    Purely voltage-driven, repeatable magnetization reversal provides a tantalizing potential for the development of spintronic devices with a minimum amount of power consumption. Substantial progress has been made in this subject especially on magnetic/ferroelectric heterostructures. Here, we report the in situ observation of such phenomenon in a NiFe thin film grown directly on a rhombohedral Pb(Mg1/3Nb2/3)0.7Ti0.3O3(PMN-PT) ferroelectric crystal. Under a cyclic voltage applied perpendicular to the PMN-PT without a magnetic field, the local magnetization of NiFe can be repetitively reversed through an out-of-plane excursion and then back into the plane. Using phase field simulations we interpret magnetization reversal as a synergistic effect of the metastable ferroelastic switching in the PMN-PT and an electrically rotatable local exchange bias field arising from the heterogeneously distributed NiO clusters at the interface.

  16. Dynamic in situ observation of voltage-driven repeatable magnetization reversal at room temperature.

    PubMed

    Gao, Ya; Hu, Jia-Mian; Nelson, C T; Yang, T N; Shen, Y; Chen, L Q; Ramesh, R; Nan, C W

    2016-01-01

    Purely voltage-driven, repeatable magnetization reversal provides a tantalizing potential for the development of spintronic devices with a minimum amount of power consumption. Substantial progress has been made in this subject especially on magnetic/ferroelectric heterostructures. Here, we report the in situ observation of such phenomenon in a NiFe thin film grown directly on a rhombohedral Pb(Mg1/3Nb2/3)0.7Ti0.3O3(PMN-PT) ferroelectric crystal. Under a cyclic voltage applied perpendicular to the PMN-PT without a magnetic field, the local magnetization of NiFe can be repetitively reversed through an out-of-plane excursion and then back into the plane. Using phase field simulations we interpret magnetization reversal as a synergistic effect of the metastable ferroelastic switching in the PMN-PT and an electrically rotatable local exchange bias field arising from the heterogeneously distributed NiO clusters at the interface. PMID:27029464

  17. Dynamic in situ observation of voltage-driven repeatable magnetization reversal at room temperature

    PubMed Central

    Gao, Ya; Hu, Jia-Mian; Nelson, C. T.; Yang, T. N.; Shen, Y.; Chen, L. Q.; Ramesh, R.; Nan, C. W.

    2016-01-01

    Purely voltage-driven, repeatable magnetization reversal provides a tantalizing potential for the development of spintronic devices with a minimum amount of power consumption. Substantial progress has been made in this subject especially on magnetic/ferroelectric heterostructures. Here, we report the in situ observation of such phenomenon in a NiFe thin film grown directly on a rhombohedral Pb(Mg1/3Nb2/3)0.7Ti0.3O3(PMN-PT) ferroelectric crystal. Under a cyclic voltage applied perpendicular to the PMN-PT without a magnetic field, the local magnetization of NiFe can be repetitively reversed through an out-of-plane excursion and then back into the plane. Using phase field simulations we interpret magnetization reversal as a synergistic effect of the metastable ferroelastic switching in the PMN-PT and an electrically rotatable local exchange bias field arising from the heterogeneously distributed NiO clusters at the interface. PMID:27029464

  18. Magnetic and velocity fluctuation measurements in the REPUTE-1 reversed-field pinch plasma

    SciTech Connect

    Ejiri, A.; Ohdachi, S.; Oikawa, T.; Shinohara, S.; Yamagishi, K.; Toyama, H.; Miyamoto, K. )

    1994-05-01

    Magnetic and velocity fluctuations are studied in the REPUTE-1 [Plasma Phys. Controlled Fusion [bold 28], 805 (1986)] reversed-field pinch (RFP). The first measurement of velocity fluctuation in an RFP plasma has been done using a Doppler shift of the O V(O[sup 4+], 278.1 nm) line. The fluctuation level increases as the radius of the viewing chord increases. Magnetic fluctuation measurements by an insertable probe reveal that the radial cross correlation of toroidal field fluctuation changes its sign at the radius slightly inside the reversal surface. The level of magnetohydrodynamic dynamo term is estimated from magnetic fluctuations at the surface correlation changes and oxygen velocity fluctuations measured with the chord distance of 115 mm. The dynamo term and that due to resistivity are the same level. This fact is consistent with Ohm's law on which magnetohydrodynamic dynamo models are based.

  19. Magnetization reversal of uncompensated Fe moments in exchangebiased Ni/FeF2 bilayers

    SciTech Connect

    Arenholz, Elke; Liu, Kai; Li, Zhipan; Schuller, Ivan K.

    2006-01-01

    The magnetization reversal of uncompensated Fe moments in exchange biased Ni/FeF{sub 2} bilayers was determined using soft x-ray magnetic circular and linear dichroism. The hysteresis loops resulting from the Fe moments are almost identical to those of the ferromagnetic Ni layer. However, a vertical loop shift indicates that some Fe moments are pinned in the antiferromagnetically ordered FeF{sub 2}. The pinned moments are oriented antiparallel to small cooling fields leading to negative exchange bias, but parallel to large cooling fields resulting in positive exchange bias. No indication for the formation of a parallel antiferromagnetic domain wall in the FeF{sub 2} layer upon magnetization reversal in the Ni layer was found.

  20. Time and temperature dependences of the magnetization reversal in a Co /Pd multilayer film

    NASA Astrophysics Data System (ADS)

    Brown, C. Scott; Harrell, J. W.; Matsunuma, S.

    2006-09-01

    The time and temperature dependences of the magnetization reversal have been measured in a high-coercivity Co /Pd multilayer film characterized by nucleation and domain wall motion. The time and field dependences of magnetic relaxation curves at room temperature were interpreted in terms of an energy barrier that depends linearly on reverse field, suggesting a Sharrock-type [M. P. Sharrock and J. T. McKinney, IEEE Trans. Magn. 17, 3020 (1981)] equation for the time and temperature dependences of coercivity with unity exponent. The sweep rate and temperature dependence of the coercivity were analyzed using the Sharrock equation to obtain the temperature dependence of the intrinsic, short-time coercivity H0 and the zero-field energy barrier E0. A single power law behavior was found for H0 versus the saturation magnetization Ms.

  1. Nucleation controlled magnetization reversal mechanism in oriented L10 FeCoPt ternary alloys

    NASA Astrophysics Data System (ADS)

    Goyal, Rajan; Sehdev, Neeru; Lamba, S.; Annapoorni, S.

    2016-01-01

    The angular dependence of scaled coercivity is investigated within the framework of various theoretical models to gather an insight into the magnetization reversal mechanism in hard magnetic materials. FeCoPt ternary alloy thin films with low concentration of Co were successfully fabricated on an <100> Si substrate with different working pressures in order to attain an optimum energy product. The structural and hysteresis curve analysis show an improvement in atomic ordering and orientation of easy axis with annealing temperature. The experimental data for angular dependence of coercivity along with the theoretical predications based on the nucleation model indicates that the dominant reversal mechanism is nucleation along with a slight contribution from pinning. The magnetic force microscopy (MFM) imaging also supports the above model. The evolution of morphology and microstructure characterized by atomic force microscopy (AFM) was directly linked to an increase in surface roughness.

  2. Reliable spin-transfer torque driven precessional magnetization reversal with an adiabatically decaying pulse

    NASA Astrophysics Data System (ADS)

    Pinna, D.; Ryan, C. A.; Ohki, T.; Kent, A. D.

    2016-05-01

    We show that a slowly decaying current pulse can lead to nearly deterministic precessional switching in the presence of noise. We consider a biaxial macrospin, with an easy axis in-plane and a hard axis out-of-plane, typical of thin film nanomagnets patterned into asymmetric shapes. Out-of-plane precessional magnetization orbits are excited with a current pulse with a component of spin polarization normal to the film plane. By numerically integrating the stochastic Landau-Lifshitz-Gilbert-Slonczewski equation we show that thermal noise leads to strong dephasing of the magnetization orbits. However, an adiabatically decreasing pulse amplitude overwhelmingly leads to magnetization reversal, with a final state dependent on the pulse polarity. We develop an analytic model to explain this phenomena and to determine the pulse decay time necessary for adiabatic magnetization relaxation and thus deterministic magnetization switching.

  3. Observations of improved confinement in field reversed configurations sustained by antisymmetric rotating magnetic fields

    SciTech Connect

    Guo, H.Y.; Hoffman, A.L.; Steinhauer, L.C.

    2005-06-15

    Rotating magnetic fields (RMF) have been employed to both form and sustain currents in field reversed configurations (FRC). A major concern about this method has been the fear of opening up magnetic field lines with even small ratios of vacuum RMF B{sub {omega}} to external confinement field B{sub e}. A recently proposed innovation was to use an antisymmetric arrangement of RMF, but vacuum calculations with full RMF penetration showed that very low values of B{sub {omega}}/B{sub e} would still be required to provide field-line closure. Recent comparisons of symmetric and antisymmetric RMF drive on the translation, confinement, and sustainment (TCS) facility [A. L. Hoffman, H. Y. Guo, J. T. Slough et al., Fusion Sci. Technol. 41, 92 (2002)] have shown strong improvements in the basic confinement properties of the FRCs when using antisymmetric drive, even with ratios of B{sub {omega}}/B{sub e} as high as 0.3. This is due to normal standard operation with only partial penetration of the RMF beyond the FRC separatrix. The uniform transverse RMF in vacuum is shielded by the conducting plasma, resulting in a mostly azimuthal field near the FRC separatrix with a very small radial component. Simple numerical calculations using analytical solutions for the partially penetrated antisymmetric RMF, superimposed on Grad-Shafranov solutions for the poloidal FRC fields, show good field-line closure for the TCS experimental conditions. The antisymmetric arrangement also leads to more efficient current drive and improved stabilization of rotational modes.

  4. Magnetic properties of ZnO nanoparticles.

    PubMed

    Garcia, M A; Merino, J M; Fernández Pinel, E; Quesada, A; de la Venta, J; Ruíz González, M L; Castro, G R; Crespo, P; Llopis, J; González-Calbet, J M; Hernando, A

    2007-06-01

    We experimentally show that it is possible to induce room-temperature ferromagnetic-like behavior in ZnO nanoparticles without doping with magnetic impurities but simply inducing an alteration of their electronic configuration. Capping ZnO nanoparticles ( approximately 10 nm size) with different organic molecules produces an alteration of their electronic configuration that depends on the particular molecule, as evidenced by photoluminescence and X-ray absorption spectroscopies and altering their magnetic properties that varies from diamagnetic to ferromagnetic-like behavior.

  5. Magnetic logging: Detection of the earth's magnetic field reversals and application to borehole magnetostratigraphy

    SciTech Connect

    Bouisset, P.; Lalanne, B.; Augustin, A. ); Pages, G. )

    1991-03-01

    TOTAL CFP and CEA (the French Atomic Energy Commission) designed and developed two magnetic logging tools for precise and reliable in-situ magnetic measurements in the low magnetized sedimentary formations encountered when drilling for oil. The tools, measuring respectively the magnetic field and the magnetic susceptibility of the rocks, are operated as standard logging tools, and logs are recorded during standard logging operations. A proper combination of these magnetic respectively the magnetic field and the magnetic susceptibility of the rocks, are operated as standard logging tools, and logs are recorded during standard logging operations. A proper combination of these magnetic measurements leads to the determination, every meter, of natural remanent magnetization polarity, from which the direction of the Earth's magnetic field at the time of sedimentation is derived. A magnetostratigraphic sequence is obtained for each well and appears to be similar to the magnetostratigraphic reference scale. Application of this method to wells in the North Sea gives good results for correlations and absolute age determination, as well as facies diachronism. Further comparison of results obtained from magnetic measurements and from sequence stratigraphy applied to conventional logs shows that third-order sequence boundaries can be diachronous in wells 80 km apart. Although the potential of magnetic measurements is still under investigation, the first encouraging results clearly show that the new dating method presented in this paper can be very helpful in petroleum geology.

  6. Magnetic and structural properties of ferrihydrite/hematite nanocomposites

    NASA Astrophysics Data System (ADS)

    Pariona, N.; Camacho-Aguilar, K. I.; Ramos-González, R.; Martinez, Arturo I.; Herrera-Trejo, M.; Baggio-Saitovitch, E.

    2016-05-01

    A rich variety of ferrihydrite/hematite nanocomposites (NCs) with specific size, composition and properties were obtained in transformation reactions of 2-line ferrihydrite. Transmission electron microscopy (TEM) observations showed that the NCs consist of clusters of strongly aggregated nanoparticles (NPs) similarly to a "plum pudding", where hematite NPs "raisins" are surrounded by ferrihydrite "pudding". Magnetic measurements of the NCs correlate very well with TEM results; i.e., higher coercive fields correspond to greater hematite crystallite size. First order reversal curve (FORC) measurements were used for the characterization of the magnetic components of the NCs. FORC diagrams revealed that the NCs prepared at short times are composed by single domains with low coercivity, and NCs prepared at times larger than 60 min exhibited elongated distribution along the Hc axis. It suggested that these samples consist of mixtures of different kinds of hematite particles, ones with low coercivity and others with coercivity greater than 600 Oe. For NCs prepared at times larger than 60 min, Mossbauer spectroscopy revealed the presence of two sextets, which one was assigned to fine hematite particles and other to hematite particles with hyperfine parameters near to bulk hematite. The correlation of the structural and magnetic properties of the ferrihydrite/hematite NCs revealed important characteristics of these materials which have not been reported elsewhere.

  7. Magnetic properties of artificially synthesized ferritins

    NASA Astrophysics Data System (ADS)

    Kim, B. J.; Lee, H. I.; Cho, S.-B.; Yoon, S.; Suh, B. J.; Jang, Z. H.; St. Pierre, T. G.; Kim, S.-W.; Kim, K.-S.

    2005-05-01

    Human ferritin homopolymers with H or L subunits (rHF and rLF) were genetically engineered in E coli. Apoferritins were then reconstituted with 2000 Fe atoms. A big difference was observed in the rates of iron uptake, whereas the mean core size was similar in rHF and rLF. Magnetization of the recombinant human ferritins were measured as functions of temperature and field. The blocking temperature TB(H) at low fields is considerably higher in rLF than in rHF. From the fit of M(H ) data to a modified Langevin function: M(H )=M0L(μpH/kBT)+χaH, the effective magnetic moment μp is found to be much larger in rLF than in rHF. Experimental data demonstrate that the magnetic properties, in particular, the uncompensated spins of ferritin core are related to the biomineralization process in ferritins.

  8. Reversible encephalopathy associated with cholesterol embolism syndrome: magnetic resonance imaging and pathological findings

    PubMed Central

    Andreux, F; Marro, B; Khoury, N EI; Seilhean, D; Alamowitch, S

    2007-01-01

    We describe a patient found to have acute diffuse and reversible encephalopathy on magnetic resonance imaging (MRI) associated with cholesterol emboli syndrome (CES). The initial MRI showed extensive white matter, basal ganglia and cortical damage without evidence of brain infarction. Dramatic clinical and MRI improvement was observed with corticosteroids. Pathologically, cholesterol crystal emboli were found in the lumen of skin and brain arteries and were associated with varying degrees of inflammation of the arteriole wall. This case suggests that CES may be responsible for extensive, acute and reversible encephalopathy underlined by an inflammation of brain arteries. PMID:17229746

  9. Magnetic Properties of Friction Stir Processed Composite

    NASA Astrophysics Data System (ADS)

    Das, Shamiparna; Martinez, Nelson Y.; Das, Santanu; Mishra, Rajiv S.; Grant, Glenn J.; Jana, Saumyadeep; Polikarpov, Evgueni

    2016-07-01

    Of the many existing inspection or monitoring systems, each has its own advantages and drawbacks. These systems are usually comprised of semi-remote sensors that frequently cause difficulty in reaching complex areas of a component. This study proposes to overcome that difficulty by developing embedded functional composites, so that embedding can be achieved in virtually any component part and periodically can be interrogated by a reading device. The "reinforcement rich" processed areas can then be used to record properties such as strain, temperature, and stress state, to name a few, depending on the reinforcement material. Friction stir processing was used to fabricate a magnetostrictive composite by embedding galfenol particles into a nonmagnetic aluminum matrix. The aim was to develop a composite that produces strain in response to a varying magnetic field. Reinforcements were distributed uniformly in the matrix. Magnetization curves were studied using a vibrating sample magnetometer. A simple and cost-effective setup was developed to measure the magnetostrictive strain of the composites. Important factors affecting the magnetic properties were identified and the processing route was modified to improve the magnetic response.

  10. Magnetic and dielectric properties of lunar samples

    NASA Technical Reports Server (NTRS)

    Strangway, D. W.; Pearce, G. W.; Olhoeft, G. R.

    1977-01-01

    Dielectric properties of lunar soil and rock samples showed a systematic character when careful precautions were taken to ensure there was no moisture present during measurement. The dielectric constant (K) above 100,000 Hz was directly dependent on density according to the formula K = (1.93 + or - 0.17) to the rho power where rho is the density in g/cc. The dielectric loss tangent was only slightly dependent on density and had values less than 0.005 for typical soils and 0.005 to 0.03 for typical rocks. The loss tangent appeared to be directly related to the metallic ilmenite content. It was shown that magnetic properties of lunar samples can be used to study the distribution of metallic and ferrous iron which shows systematic variations from soil type to soil type. Other magnetic characteristics can be used to determine the distribution of grain sizes.

  11. Magnetic Properties of CoFe_2O4 and Fe_3O_4

    NASA Astrophysics Data System (ADS)

    Rodriguez, Robert; Chan, T.; Kenning, G. G.; Huang, L.; Yan, Y.

    2002-03-01

    In order to optimize the magnetization of magnetic nanoparticles for use as Magnetic Resonance Imaging contrast agents and other in vivo biological applications, we have synthesized CoFe_2O_4(Liu, C.; Bingsuo, Z.; Rondinone, A.J.; Zhang, Z.J. J. Am. Chem. Soc.) 122, 6263 (2000). and Fe_3O_4(Shen, T.; Weissleder, R.; Papisov, M.; Bogdanov, A.; Brady, T. MRM) 29, 599 (1993). magnetic nanoparticles of sizes 5, 8, and 11nm using water-in-oil reverse micelles. Size was determined using Dynamic Light Scattering (DLS), X-Ray Diffraction (XRD), and High Pressure Liquid Chromatography (HPLC). Magnetic properties were measure from 10K-340K using SQUID magnetometry. Magnetization as a function of magnetic field has been performed at approximately body temperature ( ~310K) in order to help us determine the optimal size and composition for in vivo application.

  12. Magnetic properties of ordered NiPt

    NASA Astrophysics Data System (ADS)

    Brommer, P. E.; Franse, J. J. M.

    1988-04-01

    Thermal expansion, forced volume magnetostriction and high magnetic field data are presented on the ordered equiatomic NiPt compound. Values are derived for the magnetovolume parameter κC (≃3 × 10 -6kg2A-2m-4), and for the electronic and lattice Grüneisen parameters (Γ e ≊ 5.6; Γ latt ≊ 2.5) . Ordering effects on the magnetoelastic properties are studied for alloys containing 40-60 at % Ni.

  13. Nanoscale magnetization reversal caused by electric field-induced ion migration and redistribution in cobalt ferrite thin films.

    PubMed

    Chen, Xinxin; Zhu, Xiaojian; Xiao, Wen; Liu, Gang; Feng, Yuan Ping; Ding, Jun; Li, Run-Wei

    2015-04-28

    Reversible nanoscale magnetization reversal controlled merely by electric fields is still challenging at the moment. In this report, first-principles calculation indicates that electric field-induced magnetization reversal can be achieved by the appearance of unidirectional magnetic anisotropy along the (110) direction in Fe-deficient cobalt ferrite (CoFe(2-x)O4, CFO), as a result of the migration and local redistribution of the Co(2+) ions adjacent to the B-site Fe vacancies. In good agreement with the theoretical model, we experimentally observed that in the CFO thin films the nanoscale magnetization can be reversibly and nonvolatilely reversed at room temperature via an electrical ion-manipulation approach, wherein the application of electric fields with appropriate polarity and amplitude can modulate the size of magnetic domains with different magnetizations up to 70%. With the low power consumption (subpicojoule) characteristics and the elimination of external magnetic field, the observed electric field-induced magnetization reversal can be used for the construction of energy-efficient spintronic devices, e.g., low-power electric-write and magnetic-read memories. PMID:25794422

  14. The effects of thermally reversible agents on PVC stability properties

    NASA Astrophysics Data System (ADS)

    Wang, J.; Yao, J.; Xiong, X. H.; Jia, C. X.; Ren, R.; Chen, P.; Liu, X. M.

    2016-07-01

    One kind of thermally reversible cross-linking agents for improving PVC thermally stability was synthesized. The chemical structure and thermally reversible characteristics of cross-linking agents were investigated by FTIR and DSC analysis, respectively. FTIR results confirmed that the cyclopentadienyl barium mercaptides ((CPD-C2H4S)2Ba) were successfully synthesized. DSC results showed it has thermally reversible characteristics and the depolymerization temperature was between 170 °C and 205 °C. The effects of cross-linking reaction time on gel content of Poly(vinyl chloride) compounds was evaluated. The gel content value arrived at 42% after being cross-linked for 25 min at 180 C. The static thermally stability measurement proved that the thermally stability of PVC compounds was improved.

  15. Formation of a field reversed configuration for magnetic and electrostatic confinement of plasma

    DOEpatents

    Rostoker, Norman; Binderbauer, Michl

    2003-12-16

    A system and method for containing plasma and forming a Field Reversed Configuration (FRC) magnetic topology are described in which plasma ions are contained magnetically in stable, non-adiabatic orbits in the FRC. Further, the electrons are contained electrostatically in a deep energy well, created by tuning an externally applied magnetic field. The simultaneous electrostatic confinement of electrons and magnetic confinement of ions avoids anomalous transport and facilitates classical containment of both electrons and ions. In this configuration, ions and electrons may have adequate density and temperature so that upon collisions they are fused together by nuclear force, thus releasing fusion energy. Moreover, the fusion fuel plasmas that can be used with the present confinement system and method are not limited to neutronic fuels only, but also advantageously include advanced fuels.

  16. Formation of a field reversed configuration for magnetic and electrostatic confinement of plasma

    DOEpatents

    Rostoker, Norman; Binderbauer, Michl; Qerushi, Artan; Tahsiri, Hooshang

    2007-02-20

    A system and method for containing plasma and forming a Field Reversed Configuration (FRC) magnetic topology are described in which plasma ions are contained magnetically in stable, non-adiabatic orbits in the FRC. Further, the electrons are contained electrostatically in a deep energy well, created by tuning an externally applied magnetic field. The simultaneous electrostatic confinement of electrons and magnetic confinement of ions avoids anomalous transport and facilitates classical containment of both electrons and ions. In this configuration, ions and electrons may have adequate density and temperature so that upon collisions they are fused together by nuclear force, thus releasing fusion energy. Moreover, the fusion fuel plasmas that can be used with the present confinement system and method are not limited to neutronic fuels only, but also advantageously include advanced fuels.

  17. Formation of a field reversed configuration for magnetic and electrostatic confinement of plasma

    DOEpatents

    Rostoker, Norman; Binderbauer, Michl; Qerushi, Artan; Tahsiri, Hooshang

    2006-02-07

    A system and method for containing plasma and forming a Field Reversed Configuration (FRC) magnetic topology are described in which plasma ions are contained magnetically in stable, non-adiabatic orbits in the FRC. Further, the electrons are contained electrostatically in a deep energy well, created by tuning an externally applied magnetic field. The simultaneous electrostatic confinement of electrons and magnetic confinement of ions avoids anomalous transport and facilitates classical containment of both electrons and ions. In this configuration, ions and electrons may have adequate density and temperature so that upon collisions they are fused together by nuclear force, thus releasing fusion energy. Moreover, the fusion fuel plasmas that can be used with the present confinement system and method are not limited to neutronic fuels only, but also advantageously include advanced fuels.

  18. Domain structures and magnetization reversal in Co/Pd and CoFeB/Pd multilayers

    SciTech Connect

    Sbiaa, R.; Ranjbar, M.; Åkerman, J.

    2015-05-07

    Domain structures and magnetization reversal of (Co/Pd) and (CoFeB/Pd) multilayers with 7 and 14 repeats were investigated. The Co-based multilayers show much larger coercivities, a better squareness, and a sharper magnetization switching than CoFeB-based multilayers. From magnetic force microscopy observations, both structures show strong reduction in domains size as the number of repeats increases but the magnetic domains for Co-based multilayers are more than one order of magnitude larger than for CoFeB-based multilayers. By imaging domains at different times, breaks in the (CoFeB/Pd) multilayer stripes were observed within only few hours, while no change could be seen for (Co/Pd) multilayers. Although CoFeB single layers are suitable for magnetoresistive devices due to their large spin polarization and low damping constants, their lamination with Pd suffers mainly from thermal instability.

  19. Magnetohydrodynamic Effects in Propagating Relativistic Ejecta: Reverse Shock and Magnetic Acceleration

    NASA Technical Reports Server (NTRS)

    Mizuno, Y.; Nishikawa, K.I.; Zhang, B.; Giacomazzo, B.; Hardee, P.E.; Nagataki, S.; Hartmann, D.H.

    2008-01-01

    We solve the Riemann problem for the deceleration of arbitrarily magnetized relativistic ejecta injected into a static unmagnetized medium. We find that for the same initial Lorentz factor, the reverse shock becomes progressively weaker with increasing magnetization s (the Poynting-to-kinetic energy flux ratio), and the shock becomes a rarefaction wave when s exceeds a critical value, sc, defined by the balance between the magnetic pressure in the ejecta and the thermal pressure in the forward shock. In the rarefaction wave regime, we find that the rarefied region is accelerated to a Lorentz factor that is significantly larger than the initial value. This acceleration mechanism is due to the strong magnetic pressure in the ejecta.

  20. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Gopman, D. B.; Dennis, C. L.; Chen, P. J.; Iunin, Y. L.; Finkel, P.; Staruch, M.; Shull, R. D.

    2016-06-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices.

  1. Duffing oscillation-induced reversal of magnetic vortex core by a resonant perpendicular magnetic field

    NASA Astrophysics Data System (ADS)

    Moon, Kyoung-Woong; Chun, Byong Sun; Kim, Wondong; Qiu, Z. Q.; Hwang, Chanyong

    2014-08-01

    Nonlinear dynamics of the magnetic vortex state in a circular nanodisk was studied under a perpendicular alternating magnetic field that excites the radial modes of the magnetic resonance. Here, we show that as the oscillating frequency is swept down from a frequency higher than the eigenfrequency, the amplitude of the radial mode is almost doubled to the amplitude at the fixed resonance frequency. This amplitude has a hysteresis vs. frequency sweeping direction. Our result showed that this phenomenon was due to a Duffing-type nonlinear resonance. Consequently, the amplitude enhancement reduced the vortex core-switching magnetic field to well below 10 mT. A theoretical model corresponding to the Duffing oscillator was developed from the Landau-Lifshitz-Gilbert equation to explore the physical origin of the simulation result. This work provides a new pathway for the switching of the magnetic vortex core polarity in future magnetic storage devices.

  2. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy.

    PubMed

    Gopman, D B; Dennis, C L; Chen, P J; Iunin, Y L; Finkel, P; Staruch, M; Shull, R D

    2016-01-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices. PMID:27297638

  3. Duffing oscillation-induced reversal of magnetic vortex core by a resonant perpendicular magnetic field

    PubMed Central

    Moon, Kyoung-Woong; Chun, Byong Sun; Kim, Wondong; Qiu, Z. Q.; Hwang, Chanyong

    2014-01-01

    Nonlinear dynamics of the magnetic vortex state in a circular nanodisk was studied under a perpendicular alternating magnetic field that excites the radial modes of the magnetic resonance. Here, we show that as the oscillating frequency is swept down from a frequency higher than the eigenfrequency, the amplitude of the radial mode is almost doubled to the amplitude at the fixed resonance frequency. This amplitude has a hysteresis vs. frequency sweeping direction. Our result showed that this phenomenon was due to a Duffing-type nonlinear resonance. Consequently, the amplitude enhancement reduced the vortex core-switching magnetic field to well below 10 mT. A theoretical model corresponding to the Duffing oscillator was developed from the Landau–Lifshitz–Gilbert equation to explore the physical origin of the simulation result. This work provides a new pathway for the switching of the magnetic vortex core polarity in future magnetic storage devices. PMID:25145837

  4. Duffing oscillation-induced reversal of magnetic vortex core by a resonant perpendicular magnetic field.

    PubMed

    Moon, Kyoung-Woong; Chun, Byong Sun; Kim, Wondong; Qiu, Z Q; Hwang, Chanyong

    2014-01-01

    Nonlinear dynamics of the magnetic vortex state in a circular nanodisk was studied under a perpendicular alternating magnetic field that excites the radial modes of the magnetic resonance. Here, we show that as the oscillating frequency is swept down from a frequency higher than the eigenfrequency, the amplitude of the radial mode is almost doubled to the amplitude at the fixed resonance frequency. This amplitude has a hysteresis vs. frequency sweeping direction. Our result showed that this phenomenon was due to a Duffing-type nonlinear resonance. Consequently, the amplitude enhancement reduced the vortex core-switching magnetic field to well below 10 mT. A theoretical model corresponding to the Duffing oscillator was developed from the Landau-Lifshitz-Gilbert equation to explore the physical origin of the simulation result. This work provides a new pathway for the switching of the magnetic vortex core polarity in future magnetic storage devices. PMID:25145837

  5. Duffing oscillation-induced reversal of magnetic vortex core by a resonant perpendicular magnetic field.

    PubMed

    Moon, Kyoung-Woong; Chun, Byong Sun; Kim, Wondong; Qiu, Z Q; Hwang, Chanyong

    2014-01-01

    Nonlinear dynamics of the magnetic vortex state in a circular nanodisk was studied under a perpendicular alternating magnetic field that excites the radial modes of the magnetic resonance. Here, we show that as the oscillating frequency is swept down from a frequency higher than the eigenfrequency, the amplitude of the radial mode is almost doubled to the amplitude at the fixed resonance frequency. This amplitude has a hysteresis vs. frequency sweeping direction. Our result showed that this phenomenon was due to a Duffing-type nonlinear resonance. Consequently, the amplitude enhancement reduced the vortex core-switching magnetic field to well below 10 mT. A theoretical model corresponding to the Duffing oscillator was developed from the Landau-Lifshitz-Gilbert equation to explore the physical origin of the simulation result. This work provides a new pathway for the switching of the magnetic vortex core polarity in future magnetic storage devices.

  6. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy

    PubMed Central

    Gopman, D. B.; Dennis, C. L.; Chen, P. J.; Iunin, Y. L.; Finkel, P.; Staruch, M.; Shull, R. D.

    2016-01-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices. PMID:27297638

  7. Integral physicochemical properties of reverse micelles of sodium bis(2-ethylhexyl) sulfosuccinate (AOT)

    NASA Astrophysics Data System (ADS)

    Fedyaeva, O. A.; Shubenkova, E. G.; Poshelyuzhnaya, E. G.; Lutaeva, I. A.

    2016-08-01

    The effect the degree of hydration has on optical and electrophysical properties of water/AOT/ n-hexane system is studied. It is found that AOT reverse micelles form aggregates whose dimensions grow along with the degree of hydration and temperature. Aggregation enhances their electrical conductivity and shifts the UV spectrum of AOT reverse emulsions to the red region. Four states of water are found in the structure of AOT reverse micelles.

  8. Magnetic vortex core reversal by excitation with short bursts of an alternating field.

    PubMed

    Van Waeyenberge, B; Puzic, A; Stoll, H; Chou, K W; Tyliszczak, T; Hertel, R; Fähnle, M; Brückl, H; Rott, K; Reiss, G; Neudecker, I; Weiss, D; Back, C H; Schütz, G

    2006-11-23

    The vortex state, characterized by a curling magnetization, is one of the equilibrium configurations of soft magnetic materials and occurs in thin ferromagnetic square and disk-shaped elements of micrometre size and below. The interplay between the magnetostatic and the exchange energy favours an in-plane, closed flux domain structure. This curling magnetization turns out of the plane at the centre of the vortex structure, in an area with a radius of about 10 nanometres--the vortex core. The vortex state has a specific excitation mode: the in-plane gyration of the vortex structure about its equilibrium position. The sense of gyration is determined by the vortex core polarization. Here we report on the controlled manipulation of the vortex core polarization by excitation with small bursts of an alternating magnetic field. The vortex motion was imaged by time-resolved scanning transmission X-ray microscopy. We demonstrate that the sense of gyration of the vortex structure can be reversed by applying short bursts of the sinusoidal excitation field with amplitude of about 1.5 mT. This reversal unambiguously indicates a switching of the out-of-plane core polarization. The observed switching mechanism, which can be understood in the framework of micromagnetic theory, gives insights into basic magnetization dynamics and their possible application in data storage.

  9. Dual origin of defect magnetism in graphene and its reversible switching by molecular doping.

    PubMed

    Nair, R R; Tsai, I-L; Sepioni, M; Lehtinen, O; Keinonen, J; Krasheninnikov, A V; Castro Neto, A H; Katsnelson, M I; Geim, A K; Grigorieva, I V

    2013-01-01

    Control of magnetism by applied voltage is desirable for spintronics applications. Finding a suitable material remains an elusive goal, with only a few candidates found so far. Graphene is one of them and attracts interest because of its weak spin-orbit interaction, the ability to control electronic properties by the electric field effect and the possibility to introduce paramagnetic centres such as vacancies and adatoms. Here we show that the magnetism of adatoms in graphene is itinerant and can be controlled by doping, so that magnetic moments are switched on and off. The much-discussed vacancy magnetism is found to have a dual origin, with two approximately equal contributions; one from itinerant magnetism and the other from dangling bonds. Our work suggests that graphene's spin transport can be controlled by the field effect, similar to its electronic and optical properties, and that spin diffusion can be significantly enhanced above a certain carrier density.

  10. Tracking the individual magnetic wires' switchings in ferromagnetic nanowire arrays using the first-order reversal curves (FORC) diagram method

    NASA Astrophysics Data System (ADS)

    Dobrotă, Costin-Ionuţ; Stancu, Alexandru

    2015-01-01

    The complex hysteretic properties observed in structured ferromagnetic materials can be revealed with remarkable details in magnetization processes like the first-order reversal curves (FORC) - a characterization technique extensively used in recent years. The really fundamental problem in the analysis of experimental FORC diagrams is related to the possibility to link the hysteretic properties of real physical entities in a unique way with regions from the FORC distributions. Actually, what many scientists are often doing is to use a Preisach-type interpretation of FORC data without a proof for the accuracy of this procedure. In this paper we analyze in detail the relation between the switching events of physical entities given by the Preisach function and the FORC distribution in magnetic nanowire arrays with the aim to show the limits of the conventional interpretation of FORC data. For this type of sample we show how the real switching events are contributing to the experimental diagram. We present in a systematic manner the way in which the switchings of the physical wires are observed multiple times (both as positive or negative contributions). The multiplicity of switching occurrences is not the same for all the wires in the sample, being dependent on the wire intrinsic coercivity and its position in the array. In this manner one can track the switchings contributions of real magnetic wires on the FORC diagram.

  11. Time-reversal breaking and spin transport induced by magnetic impurities in a 2D topological insulator

    NASA Astrophysics Data System (ADS)

    Derakhshan, V.; Ketabi, S. A.; Moghaddam, A. G.

    2016-09-01

    We employed the formalism of bond currents, expressed in terms of non-equilibrium Green’s function to obtain the local currents and transport features of zigzag silicene ribbon in the presence of magnetic impurity. When only intrinsic and Rashba spin-orbit interactions are present, silicene behaves as a two-dimensional topological insulator with gapless edge states. But in the presence of finite intrinsic spin-orbit interaction, the edge states start to penetrate into the bulk of the sample by increasing Rashba interaction strength. The exchange interaction induced by local impurities breaks the time-reversal symmetry of the gapless edge states and influences the topological properties strongly. Subsequently, the singularity of partial Berry curvature disappears and the silicene nanoribbon becomes a trivial insulator. On the other hand, when the concentration of the magnetic impurities is low, the edge currents are not affected significantly. In this case, when the exchange field lies in the x-y plane, the spin mixing around magnetic impurity is more profound rather than the case in which the exchange field is directed along the z-axis. Nevertheless, when the exchange field of magnetic impurities is placed in the x-y plane, a spin-polarized conductance is observed. The resulting conductance polarization can be tuned by the concentration of the impurities and even completely polarized spin transport is achievable.

  12. Time-reversal breaking and spin transport induced by magnetic impurities in a 2D topological insulator

    NASA Astrophysics Data System (ADS)

    Derakhshan, V.; Ketabi, S. A.; Moghaddam, A. G.

    2016-09-01

    We employed the formalism of bond currents, expressed in terms of non-equilibrium Green’s function to obtain the local currents and transport features of zigzag silicene ribbon in the presence of magnetic impurity. When only intrinsic and Rashba spin–orbit interactions are present, silicene behaves as a two-dimensional topological insulator with gapless edge states. But in the presence of finite intrinsic spin–orbit interaction, the edge states start to penetrate into the bulk of the sample by increasing Rashba interaction strength. The exchange interaction induced by local impurities breaks the time-reversal symmetry of the gapless edge states and influences the topological properties strongly. Subsequently, the singularity of partial Berry curvature disappears and the silicene nanoribbon becomes a trivial insulator. On the other hand, when the concentration of the magnetic impurities is low, the edge currents are not affected significantly. In this case, when the exchange field lies in the x–y plane, the spin mixing around magnetic impurity is more profound rather than the case in which the exchange field is directed along the z-axis. Nevertheless, when the exchange field of magnetic impurities is placed in the x–y plane, a spin-polarized conductance is observed. The resulting conductance polarization can be tuned by the concentration of the impurities and even completely polarized spin transport is achievable.

  13. Micromagnetic study of exchange interaction effect on magnetization reversal mode of CoFeAl

    NASA Astrophysics Data System (ADS)

    Azizah, Umi Muflihatun Nurul; Trihandaru, Suryasatriya; Wibowo, Nur Aji

    2016-02-01

    A magnetization switching dynamics of perpendicular magnetic anisotropy material CoFeAl has been simulated. This simulation was conducted using Landau-Lifshift Gilbert equation. The used magnetic parameters are magnetic anisotropy 2.3 × 106 erg/cm3, magnetic saturation 10 kG, medium Gilbert damping 0.3 and various exchange constants in a range of (1.5 - 4.0) × 10-7 erg/cm. CoFeAl is modeled as a parallel-pipe with the dimension is 50 × 50 × 20 nm3. As a result, this simulation predicts that the chosen materials exhibit good thermal stability which is greatly affected by exchange energy. Magnetization reversal mechanism is dominated by domain wall propagation process. Moreover, the simultaneous distribution of thermal with external magnetic field on the materials reduces the writing field which reaches the minimum value when exchange constant is 3.5 × 10-7 erg/cm.

  14. Local and nonlocal anisotropic transport in reversed shear magnetic fields: shearless Cantori and nondiffusive transport.

    PubMed

    Blazevski, Daniel; del-Castillo-Negrete, Diego

    2013-06-01

    A study of anisotropic heat transport in reversed shear (nonmonotonic q-profile) magnetic fields is presented. The approach is based on a recently proposed Lagrangian-Green's function method that allows an efficient and accurate integration of the parallel (i.e., along the magnetic field) heat transport equation. The magnetic field lines are described by a nontwist Hamiltonian system, known to exhibit separatrix reconnection and robust shearless (dq/dr=0) transport barriers. The changes in the magnetic field topology due to separatrix reconnection lead to bifurcations in the equilibrium temperature distribution. For perturbations of moderate amplitudes, magnetic chaos is restricted to bands flanking the shearless region. As a result, the temperature flattens in the chaotic bands and develops a very sharp radial gradient at the shearless region. For perturbations with larger amplitude, shearless Cantori (i.e., critical magnetic surfaces located at the minimum of the q profile) give rise to anomalous temperature relaxation involving widely different time scales. The first stage consists of the relatively fast flattening of the radial temperature profile in the chaotic bands with negligible flux across the shearless region that, for practical purposes, on a short time scale acts as an effective transport barrier despite the lack of magnetic flux surfaces. In the long-time scale, heat starts to flow across the shearless region, albeit at a comparatively low rate. The transport of a narrow temperature pulse centered at the reversed shear region exhibits weak self-similar scaling with non-Gaussian scaling functions indicating that transport at this scale cannot be modeled as a diffusive process with a constant diffusivity. Evidence of nonlocal effective radial transport is provided by the existence of regions with nonzero heat flux and zero temperature gradient. Parametric flux-gradient plots exhibit multivalued loops that question the applicability of the Fourier

  15. Intrinsic torque reversals induced by magnetic shear effects on the turbulence spectrum in tokamak plasmas

    SciTech Connect

    Lu, Z. X.; Wang, W. X.; Diamond, P. H.; Tynan, G.; Ethier, S.; Gao, C.; Rice, J.

    2015-05-04

    We report that intrinsic torque, which can be generated by turbulent stresses, can induce toroidal rotation in a tokamak plasma at rest without direct momentum injection. Reversals in intrinsic torque have been inferred from the observation of toroidal velocity changes in recent lower hybrid current drive (LHCD) experiments. Here we focus on understanding the cause of LHCD-induced intrinsic torque reversal using gyrokinetic simulations and theoretical analyses. A new mechanism for the intrinsic torque reversal linked to magnetic shear (sˆ) effects on the turbulence spectrum is identified. This reversal is a consequence of the ballooning structure at weak sˆ . Based on realistic profiles from the Alcator C-Mod LHCD experiments, simulations demonstrate that the intrinsic torque reverses for weak sˆ discharges and that the value of sˆ crit is consistent with the experimental results sˆ expcrit [Rice et al., Phys. Rev. Lett. 111, 125003 (2013)]. In conclusion, the consideration of this intrinsic torque feature in our work is important for the understanding of rotation profile generation at weak and its consequent impact on macro-instability stabilization and micro-turbulence reduction, which is crucial for ITER. It is also relevant to internal transport barrier formation at negative or weakly positive sˆ .

  16. Intrinsic torque reversals induced by magnetic shear effects on the turbulence spectrum in tokamak plasmas

    SciTech Connect

    Lu, Z. X.; Tynan, G.; Wang, W. X.; Ethier, S.; Diamond, P. H.; Gao, C.; Rice, J.

    2015-05-15

    Intrinsic torque, which can be generated by turbulent stresses, can induce toroidal rotation in a tokamak plasma at rest without direct momentum injection. Reversals in intrinsic torque have been inferred from the observation of toroidal velocity changes in recent lower hybrid current drive (LHCD) experiments. This work focuses on understanding the cause of LHCD-induced intrinsic torque reversal using gyrokinetic simulations and theoretical analyses. A new mechanism for the intrinsic torque reversal linked to magnetic shear (s{sup ^}) effects on the turbulence spectrum is identified. This reversal is a consequence of the ballooning structure at weak s{sup ^}. Based on realistic profiles from the Alcator C-Mod LHCD experiments, simulations demonstrate that the intrinsic torque reverses for weak s{sup ^} discharges and that the value of s{sup ^}{sub crit} is consistent with the experimental results s{sup ^}{sub crit}{sup exp}≈0.2∼0.3 [Rice et al., Phys. Rev. Lett. 111, 125003 (2013)]. The consideration of this intrinsic torque feature in our work is important for the understanding of rotation profile generation at weak s{sup ^} and its consequent impact on macro-instability stabilization and micro-turbulence reduction, which is crucial for ITER. It is also relevant to internal transport barrier formation at negative or weakly positive s{sup ^}.

  17. Magnetic properties of nano-composite particles

    NASA Astrophysics Data System (ADS)

    Xu, Xia

    Chemical synthesis routes for hollow spherical BaFe12O 19, hollow mesoporous spherical BaFe12O19, worm-shape BaFe12O19 and FeCo particles were developed. These structured particles have great potentials for the applications including magnetic recording medium, catalyst support, and energy storage. Magnetically exchange coupled hard/soft SrFe12O19/FeCo and MnBi/FeCo composites were synthesized through a newly proposed process of magnetic self-assembly. These exchange coupled composites can be potentially used as rare-earth free permanent magnets. Hollow spherical BaFe12O19 particles (shell thickness ˜5 nm) were synthesized from eth-ylene glycol assisted spray pyrolysis. Hollow mesoporous spherical BaFe12O19 particles (shell thickness ˜100 nm) were synthesized from ethanol assisted spray pyrolysis, followed by alkaline ethylene glycol etching at 185 °C. An alpha-Fe2O3 and BaCO3 nanoparticle mixture was synthesized with reverse microemulsion, followed by annealing at 900 °C for 2 hours to get worm-shape BaFe 12O19 particles, which consisted of 3-7 stacked hexagonal plates. FeCo nanoparticles were synthesized by reducing FeCl2 and CoCl2 in diphenyl ether with n-butyllithium at 200 °C in an inert gas environment. The surfactant of oleic acid was used in the synthesis to make particles well dispersed in nonpolar solvents (such as hexane). SrFe12O19/FeCo core/shell particles were prepared through a magnetic self-assembly process. The as-synthesized soft FeCo nanoparticles were magnetically attracted by hard SrFe12O19 parti-cles, forming a SrFe12O19/FeCo core/shell structure. The magnetic self-assembly mechanism was confirmed by applying alternating-current demagnetization to the core/shell particles, which re-sulted in a separation of SrFe 12O19 and FeCo particles. MnBi/FeCo composites were synthesized, and the exchange coupling between MnBi and FeCo phases was demonstrated by smooth magnetic hysteresis loop of MnBi/FeCo composites. The thermal stability of Mn

  18. Effects of terbium sulfide addition on magnetic properties, microstructure and thermal stability of sintered Nd-Fe-B magnets

    NASA Astrophysics Data System (ADS)

    Xiang-Bin, Li; Shuo, Liu; Xue-Jing, Cao; Bei-Bei, Zhou; Ling, Chen; A-Ru, Yan; Gao-Lin, Yan

    2016-07-01

    To increase coercivity and thermal stability of sintered Nd-Fe-B magnets for high-temperature applications, a novel terbium sulfide powder is added into (Pr0.25Nd0.75)30.6Cu0.15FebalB1 (wt.%) basic magnets. The effects of the addition of terbium sulfide on magnetic properties, microstructure, and thermal stability of sintered Nd-Fe-B magnets are investigated. The experimental results show that by adding 3 wt.% Tb2S3, the coercivity of the magnet is remarkably increased by about 54% without a considerable reduction in remanence and maximum energy product. By means of the electron probe microanalyzer (EPMA) technology, it is observed that Tb is mainly present in the outer region of 2:14:1 matrix grains and forms a well-developed Tb-shell phase, resulting in enhancement of H A, which accounts for the coercivity enhancement. Moreover, compared with Tb2S3-free magnets, the reversible temperature coefficients of remanence (α) and coercivity (β) and the irreversible flux loss of magnetic flow (h irr) values of Tb2S3-added magnets are improved, indicating that the thermal stability of the magnets is also effectively improved. Project supported by the Science Funds from the Ministry of Science and Technology, China (Grant Nos. 2014DFB50130 and 2011CB612304) and the National Natural Science Foundation of China (Grant Nos. 51172168 and 51072139).

  19. Magnetic properties of iron minerals produced by natural iron- and manganese-reducing groundwater bacteria

    NASA Astrophysics Data System (ADS)

    Abrajevitch, Alexandra; Kondratyeva, Lubov M.; Golubeva, Evgeniya M.; Kodama, Kazuto; Hori, Rie S.

    2016-06-01

    Understanding the contribution of biogenic magnetic particles into sedimentary assemblages is a current challenge in paleomagnetism. It has been demonstrated recently that magnetic particles produced through biologically controlled mineralization processes, such as magnetosomes from magnetotactic bacteria, contribute to the recording of natural remanent magnetization in marine and lacustrian sediments. Contributions from other, biologically induced, mineralization types, which are known from multiple laboratory experiments to include magnetic minerals, remain largely unknown. Here, we report magnetic properties of iron minerals formed by a community of iron- and manganese-reducing bacteria isolated from a natural groundwater deposit during a two year long incubation experiment. The main iron phases of the biomineralized mass are lepidocrocite, goethite and magnetite, each of which has environmental significance. Unlike the majority of the previous studies that reported superparamagnetic grain size, and thus no remanence carrying capacity of biologically induced magnetite, hysteresis and first order reversal curves measurements in our study have not detected significant superparamagnetic contribution. The biomineralized mass, instead, contains a mixture of single-domain to pseudo-single-domain and multi-domain magnetite particles that are capable of carrying a stable chemical remanent magnetization. Isothermal remanent magnetization acquisition parameters and first order reversal curves signatures of the biomineralized samples deviate from previously proposed criteria for the distinction of extracellular (biologically induced) magnetic particles in mixtures. Given its potential significance as a carrier of natural remanent magnetization, environmental requirements, distribution in nature and the efficiency in the geomagnetic field recording by biologically induced mineralization need comprehensive investigation.

  20. Magnetic properties of iron minerals produced by natural iron- and manganese-reducing groundwater bacteria

    NASA Astrophysics Data System (ADS)

    Abrajevitch, Alexandra; Kondratyeva, Lubov M.; Golubeva, Evgeniya M.; Kodama, Kazuto; Hori, Rie S.

    2016-08-01

    Understanding the contribution of biogenic magnetic particles into sedimentary assemblages is a current challenge in palaeomagnetism. It has been demonstrated recently that magnetic particles produced through biologically controlled mineralization processes, such as magnetosomes from magnetotactic bacteria, contribute to the recording of natural remanent magnetization in marine and lacustrian sediments. Contributions from other, biologically induced, mineralization types, which are known from multiple laboratory experiments to include magnetic minerals, remain largely unknown. Here, we report magnetic properties of iron minerals formed by a community of iron- and manganese-reducing bacteria isolated from a natural groundwater deposit during a 2 yr long incubation experiment. The main iron phases of the biomineralized mass are lepidocrocite, goethite and magnetite, each of which has environmental significance. Unlike the majority of the previous studies that reported superparamagnetic grain size, and thus no remanence carrying capacity of biologically induced magnetite, hysteresis and first-order reversal curves measurements in our study have not detected significant superparamagnetic contribution. The biomineralized mass, instead, contains a mixture of single-domain to pseudo-single-domain and multidomain magnetite particles that are capable of carrying a stable chemical remanent magnetization. Isothermal remanent magnetization acquisition parameters and first-order reversal curves signatures of the biomineralized samples deviate from previously proposed criteria for the distinction of extracellular (biologically induced) magnetic particles in mixtures. Given its potential significance as a carrier of natural remanent magnetization, environmental requirements, distribution in nature and the efficiency in the geomagnetic field recording by biologically induced mineralization need comprehensive investigation.

  1. Magnetic detection and characterization of biogenic magnetic minerals: A comparison of ferromagnetic resonance and first-order reversal curve diagrams

    NASA Astrophysics Data System (ADS)

    Chang, L.; Roberts, A. P.; Winklhofer, M.; Heslop, D.; Dekkers, M. J.; Krijgsman, W.

    2014-12-01

    Biogenic magnetic minerals produced by magnetotactic bacteria occur ubiquitously in natural aquatic environments. Their identification and characterization are important for interpretation of paleomagnetic and environmental magnetic records. We compare two magnetic methods for their identification and characterization in a diverse set of sedimentary environments: ferromagnetic resonance (FMR) spectroscopy and first-order reversal curve (FORC) diagrams, constrained by transmission electron microscope observations. The advantages and limitations of each method are evaluated. FMR analysis provides a strong diagnostic indicator because of its ability to detect the strong shape anisotropy that arises from the biogenic chain architecture, but it can be obscured in mixed magnetic mineral assemblages. We develop a new FMR fitting approach that enables separation and characterization of biogenic components in natural samples. FMR spectral fitting on magnetofossil-bearing samples does not always reveal a strong signature of biogenic magnetite with <111>-aligned chains, in contrast to whole MTB cells. This indicates that strictly <111>-aligned chains are not as common in magnetofossil assemblages, either due to chain collapse or different crystallographic axis orientations. FORC analysis provides an excellent tool for isolating the biogenic component as a 'central ridge' signature with peak switching field distribution between ~20 and 60 mT. We also analyzed tuff samples with similar FMR characteristics to biogenic magnetite chains, which can cause ambiguity. We propose a magnetic protocol to improve the robustness and efficiency of biogenic magnetite identification and past microbial activity in a wide range of environments.

  2. Magnetic detection and characterization of biogenic magnetic minerals: A comparison of ferromagnetic resonance and first-order reversal curve diagrams

    NASA Astrophysics Data System (ADS)

    Chang, Liao; Roberts, Andrew P.; Winklhofer, Michael; Heslop, David; Dekkers, Mark J.; Krijgsman, Wout; Fitz Gerald, John D.; Smith, Paul

    2014-08-01

    Biogenic magnetic minerals produced by magnetotactic bacteria occur ubiquitously in natural aquatic environments. Their identification and characterization are important for interpretation of paleomagnetic and environmental magnetic records. We compare two magnetic methods for their identification and characterization in a diverse set of sedimentary environments: ferromagnetic resonance (FMR) spectroscopy and first-order reversal curve (FORC) diagrams, constrained by transmission electron microscope observations. The advantages and limitations of each method are evaluated. FMR analysis provides a strong diagnostic indicator because of its ability to detect the strong shape anisotropy that arises from the biogenic chain architecture, but it can be obscured in mixed magnetic mineral assemblages. We develop a new FMR fitting approach that enables separation and characterization of biogenic components in natural samples. FMR spectral fitting on magnetofossil-bearing samples does not always reveal a strong signature of biogenic magnetite with <111>-aligned chains, in contrast to whole magnetotactic bacteria cells. This indicates that strictly <111>-aligned chains are not as common in magnetofossil assemblages, due to either chain collapse or different crystallographic axis orientations. FORC analysis provides an excellent tool for isolating the biogenic component as a "central ridge" signature with peak switching field distribution between ~20 and 60 mT. We also analyzed tuff samples with similar FMR characteristics to biogenic magnetite chains, which can cause ambiguity. We propose a magnetic protocol to improve the robustness and efficiency of biogenic magnetite identification and past microbial activity in a wide range of environments.

  3. A measurement setup for acquiring the local magnetic properties of plastically deformed soft magnetic materials

    SciTech Connect

    Bi Shasha; Sutor, Alexander; Lerch, Reinhard; Xiao Yunshi

    2011-04-01

    This paper introduces a new measurement setup for extraction of the local magnetic properties. With the help of finite element method simulations, modifications are made on the previous double-C-yoke method. Small dimension measuring coils are applied in the stray field produced by the magnetic circuit to evaluate the local magnetic properties of the specified part of the specimen. Through the measurements with the plastically deformed materials at different temperatures, it indicates that the magnetic properties of soft magnetic materials are quite sensitive to plastic straining. After high-temperature thermal treatment on the plastically deformed specimen, the local magnetic properties exhibit an obvious recovery.

  4. Precessional reversal in orthogonal spin transfer magnetic random access memory devices

    NASA Astrophysics Data System (ADS)

    Liu, H.; Bedau, D.; Backes, D.; Katine, J. A.; Kent, A. D.

    2012-07-01

    Single-shot time-resolved resistance measurements have been used to determine the magnetization reversal mechanisms of orthogonal spin transfer magnetic random access memory (OST-MRAM) devices at nanosecond time scales. There is a strong asymmetry between antiparallel (AP) to parallel (P) and P to AP transitions under the same pulse conditions. P to AP transitions are shown to occur by precession of the free layer magnetization, while the AP to P transition is typically direct, occurring in less than 200 ps. We associate the asymmetry with spin torques perpendicular to the plane of the free layer, an important characteristic of OST-MRAM bit cells that can be used to optimize device performance.

  5. Influence of thermal agitation on the electric field induced precessional magnetization reversal with perpendicular easy axis

    SciTech Connect

    Cheng, Hongguang Deng, Ning

    2013-12-15

    We investigated the influence of thermal agitation on the electric field induced precessional magnetization switching probability with perpendicular easy axis by solving the Fokker-Planck equation numerically with finite difference method. The calculated results show that the thermal agitation during the reversal process crucially influences the switching probability. The switching probability can be achieved is only determined by the thermal stability factor Δ of the free layer, it is independent on the device dimension, which is important for the high density device application. Ultra-low error rate down to the order of 10{sup −9} can be achieved for the device of thermal stability factor Δ of 40. Low damping factor α material should be used for the free layer for high reliability device applications. These results exhibit potential of electric field induced precessional magnetization switching with perpendicular easy axis for ultra-low power, high speed and high density magnetic random access memory (MRAM) applications.

  6. Time-Resolved AMR measurements of current induced magnetization reversal in ferromagnetic nanowires

    NASA Astrophysics Data System (ADS)

    Guittienne, Ph.; Wegrowe, J.-E.; Kelly, D.; Ansermet, J.-Ph.

    2001-03-01

    Time-resolved detection of the magnetization switching in static magnetic fields was achieved by pulsing current densities of about 107 A/cm2 in single isolated Nickel nanowires (80nm in diameter, 6000 nm in length, electrodeposited in porous membranes), using a Weathstone bridge of a 1GHz bandwidth. This irreversible transition is found to occur in a time of about 10 ns. The time of switching within the pulse, tsw, is measured as a function of applied field and current. The temperature rise due to Joule heating is deduced from the change in resistance. The entire set of data tsw(H,T) are fitted with a simple activation law, with the energy barrier height as the unique fitting parameter. The results show a strong departure from pure thermal activation indicating a current-induced magnetization reversal.

  7. Shearless bifurcation on symplectic maps of magnetic field lines in tokamaks with reversed current

    NASA Astrophysics Data System (ADS)

    Bartoloni, B.; Schelin, A. B.; Caldas, I. L.

    2016-07-01

    We introduce two-dimensional symplectic maps to describe the Poincaré maps of magnetic field lines in large aspect ratio tokamak equilibria with reversed non-monotonic plasma current density profiles. For these maps, we investigate the effect of the symmetry breaking due to the toroidal correction with a peculiar invariant, namely, a magnetic surface with a null rotation number, enclosing a vanishing current. We find that this rotationless invariant surface is surrounded by many small island chains. Furthermore, near such invariant, the symmetry breaking gives rise to two magnetic shearless invariants surrounded by twin island chains. We also find chaotic lines adjacent to all the observed islands created by the considered structurally unstable equilibria.

  8. Preparation of lipase-coated, stabilized, hydrophobic magnetic particles for reversible conjugation of biomacromolecules.

    PubMed

    Marciello, Marzia; Bolivar, Juan M; Filice, Marco; Mateo, Cesar; Guisan, Jose M

    2013-03-11

    This Communication presents the development of a novel strategy for the easy conjugation of biomolecules to hydrophobic magnetic microparticles via reversible coating with previously functionalized lipase molecules. First, the ability of lipase to be strongly adsorbed onto hydrophobic surfaces was exploited for the stabilization of microparticles in aqueous medium by the creation of a hydrophilic surface. Second, the surface amino acids of lipase can be tailored to suit biomolecule conjugation. This approach has been demonstrated by amino-epoxy activation of lipase, enabling the conjugation of different biomolecules to the magnetic particle's surface. For example, it was possible to immobilize 70% of Escherichia coli proteins on the recovered particles. Furthermore, this strategy could be extended to other lipase chemical modification protocols, enabling fine control of biomolecule coupling. These conjugation techniques constitute a modular methodology that also permits the recycling of the magnetic carrier following use.

  9. Nonvolatile, reversible electric-field controlled switching of remanent magnetization in multifunctional ferromagnetic/ferroelectric hybrids

    NASA Astrophysics Data System (ADS)

    Brandlmaier, A.; Geprägs, S.; Woltersdorf, G.; Gross, R.; Goennenwein, S. T. B.

    2011-08-01

    In spin-mechanics, the magnetoelastic coupling in ferromagnetic/ferroelectric hybrid devices is exploited in order to realize an electric-voltage control of magnetization orientation. To this end, different voltage-induced elastic strain states are used to generate different magnetization orientations. In our approach, we take advantage of the hysteretic expansion and contraction of a commercial piezoelectric actuator as a function of electrical voltage to deterministically select one of two electro-remanent elastic strain states. We investigate the resulting magnetic response in a nickel thin film/piezoelectric actuator hybrid device at room temperature, using simultaneous magneto-optical Kerr effect and magnetotransport measurements. The magnetic properties of the hybrid can be consistently described in a macrospin model, i.e., in terms of a single magnetic domain. At zero external magnetic field, the magnetization orientation in the two electro-remanent strain states differs by 15°, which corresponds to a magnetoresistance change of 0.5%. These results demonstrate that the spin-mechanics scheme indeed enables a nonvolatile electrically read- and writable memory bit where the information is encoded in a magnetic property.

  10. On a Possibility of Shock-Induced and Irradiation-Induced Self-Reversal of Magnetization in Meteorites and Impactites

    NASA Astrophysics Data System (ADS)

    Bezaeva, N. S.

    2016-08-01

    We showed using numerical modeling a possibility of impact-induced and irradiation-induced self-reversal of magnetization in ferrimagnetic minerals of terrestrial rocks and meteorites. Such phenomena are likely to be discovered in a laboratory.

  11. Magnetic molecularly imprinted polymers synthesized by surface-initiated reversible addition-fragmentation chain transfer polymerization for the enrichment and determination of synthetic estrogens in aqueous solution.

    PubMed

    Chen, Fangfang; Zhang, Jingjing; Wang, Minjun; Kong, Jie

    2015-08-01

    Magnetic molecularly imprinted polymers have attracted significant interest because of their multifunctionality of selective recognition of target molecules and rapid magnetic response. In this contribution, magnetic molecularly imprinted polymers were synthesized via surface-initiated reversible addition addition-fragmentation chain transfer polymerization using diethylstilbestrol as the template for the enrichment of synthetic estrogens. The uniform imprinted surface layer and the magnetic property of the magnetic molecularly imprinted polymers favored a fast binding kinetics and rapid analysis of target molecules. The static and selective binding experiments demonstrated a desirable adsorption capacity and good selectivity of the magnetic molecularly imprinted polymers in comparison to magnetic non-molecularly imprinted polymers. Accordingly, a corresponding analytical method was developed in which magnetic molecularly imprinted polymers were employed as magnetic solid-phase extraction materials for the concentration and determination of four synthetic estrogens (diethylstilbestrol, hexestrol, dienestrol, and bisphenol A) in fish pond water. The recoveries of these synthetic estrogens in spiked fish pond water samples ranged from 61.2 to 99.1% with a relative standard deviation of lower than 6.3%. This study provides a versatile approach to prepare well-defined magnetic molecularly imprinted polymers sorbents for the analysis of synthetic estrogens in water solution. PMID:25989155

  12. Bromelain reversibly inhibits invasive properties of glioma cells.

    PubMed

    Tysnes, B B; Maurer, H R; Porwol, T; Probst, B; Bjerkvig, R; Hoover, F

    2001-01-01

    Bromelain is an aqueous extract from pineapple stem that contains proteinases and exhibits pleiotropic therapeutic effects, i.e., antiedematous, antiinflammatory, antimetastatic, antithrombotic, and fibrinolytic activities. In this study, we tested bromelain's effects on glioma cells to assess whether bromelain could be a potential contributor to new antiinvasive strategies for gliomas. Several complementary assays demonstrated that bromelain significantly and reversibly reduced glioma cell adhesion, migration, and invasion without affecting cell viability, even after treatment periods extending over several months. Immunohistochemistry and immunoblotting experiments demonstrated that alpha3 and beta1 integrin subunits and hyaluronan receptor CD44 protein levels were reduced within 24 hours of bromelain treatment. These effects were not reflected at the RNA level because RNA profiling did not show any significant effects on gene expression. Interestingly, metabolic labelling with 35-S methionine demonstrated that de novo protein synthesis was greatly attenuated by bromelain, in a reversible manner. By using a transactivating signaling assay, we found that CRE-mediated signaling processes were suppressed. These results indicate that bromelain exerts its antiinvasive effects by proteolysis, signaling cascades, and translational attenuation.

  13. Bromelain Reversibly Inhibits Invasive Properties of Glioma Cells

    PubMed Central

    Tysnes, Berit B; Maurer, H Rainer; Porwol, Torsten; Probst, Beatrice; Bjerkvig, Rolf; Hoover, Frank

    2001-01-01

    Abstract Bromelain is an aqueous extract from pineapple stem that contains proteinases and exhibits pleiotropic therapeutic effects, i.e., antiedematous, antiinflammatory, antimetastatic, antithrombotic, and fibrinolytic activities. In this study, we tested bromelain's effects on glioma cells to assess whether bromelain could be a potential contributor to new antiinvasive strategies for gliomas. Several complementary assays demonstrated that bromelain significantly and reversibly reduced glioma cell adhesion, migration, and invasion without affecting cell viability, even after treatment periods extending over several months. Immunohistochemistry and immunoblotting experiments demonstrated that α3 and β1 integrin subunits and hyaluronan receptor CD44 protein levels were reduced within 24 hours of bromelain treatment. These effects were not reflected at the RNA level because RNA profiling did not show any significant effects on gene expression. Interestingly, metabolic labelling with 35-S methionine demonstrated that de novo protein synthesis was greatly attenuated by bromelain, in a reversible manner. By using a trans-activating signaling assay, we found that CRE-mediated signaling processes were suppressed. These results indicate that bromelain exerts its antiinvasive effects by proteolysis, signaling cascades, and translational attenuation. PMID:11774029

  14. The symmetry properties of planetary magnetic fields

    SciTech Connect

    Raedler, K.H. ); Ness, N.F. )

    1990-03-01

    This paper provides a comparative study of the geometrical structures of the magnetic fields of Earth, Jupiter, Saturn, and Uranus, starting from the traditional multipolar representations of these fields. For Earth, Jupiter, and Saturn the centered dipole, quadrupole, and octupole contributions are included, while at Uranus, only the dipole and quadrupole contributoins are considered. The magnetic fields are analyzed by decomposing them into those parts which have simple symmetry properties with respect to the rotation axis and the equatorial plane. It is found that there are a number of common features of the magnetic fields of Earth and Jupiter. Compared to Earth and Jupiter, the Saturnian field exhibits not only a high degree of symmetry about the rotation axis, by now rather well known, but also a high degree of antisymmetry about the equatorial plane. The Uranian field shows strong deviations from both such symmetries. Nevertheless, there remain features common to all four planets. The implications of these results for dynamo models are discussed. With a vgiew to Cowling's theorem the symmetry of the fields is investigated with respect to not only the rotation axis but also to other axes intersecting the plaentary center. Surprisingly, the high degree of asymmetry of the Uranian field that is observed with respect to the rotation axis reduces considerably to being compare to that for Earth or Jupiter when the appropriate axis is employed.

  15. A strong angular dependence of magnetic properties of magnetosome chains: Implications for rock magnetism and paleomagnetism

    NASA Astrophysics Data System (ADS)

    Li, Jinhua; Ge, Kunpeng; Pan, Yongxin; Williams, Wyn; Liu, Qingsong; Qin, Huafeng

    2013-10-01

    Single-domain magnetite particles produced by magnetotactic bacteria (magnetosomes) and aligned in chains are of great interest in the biosciences and geosciences. Here, we investigated angular variation of magnetic properties of aligned Magnetospirillum magneticum AMB-1 cells, each of which contains one single fragmental chain of magnetosomes. With measurements at increasing angles from the chain direction, we observed that (i) the hysteresis loop gradually changes from nearly rectangular to a ramp-like shape (e.g., Bc and remanence decrease), (ii) the acquisition and demagnetization curves of IRM shift toward higher fields (e.g., Bcr increases), and (iii) the FORC diagram shifts toward higher coercivity fields (e.g., Bc,FORC increases). For low-temperature results, compared to unoriented samples, the samples containing aligned chains have a much lower remanence loss of field-cooled (δFC) and zero-field-cooled (δZFC) remanence upon warming through the Verwey transition, higher δ-ratio (δ = δFC/δZFC) for the measurement parallel to the chain direction, and lower δ-ratio, larger δFC and δZFC values for the perpendicular measurement. Micromagnetic simulations confirm the experimental observations and reveal that the magnetization reversal of magnetosome chain appears to be noncoherent at low angles and coherent at high angles. The simulations also demonstrate that the angular dependence of magnetic properties is related to the dispersion degree of individual chains, indicating that effects of anisotropy need to be accounted for when using rock magnetism to identify magnetosomes or magnetofossils once they have been preserved in aligned chains. Additionally, this study experimentally demonstrates an empirical correspondence of the parameter Bc,FORC to Bcr rather than Bc, at least for magnetite chains with strong shape anisotropy. This suggests FORC analysis is a good discriminant of magnetofossils in sediments and rocks.

  16. Reverse shock emission driven by post-merger millisecond magnetar winds: Effects of the magnetization parameter

    NASA Astrophysics Data System (ADS)

    Liu, L. D.; Wang, L. J.; Dai, Z. G.

    2016-08-01

    The study of short-duration gamma-ray bursts provides growing evidence that a good fraction of double neutron star mergers lead to the formation of stable millisecond magnetars. The launch of Poynting flux by the millisecond magnetars could leave distinct electromagnetic signatures that reveal the energy dissipation processes in the magnetar wind. In previous studies, we assume that the magnetar wind becomes completely lepton-dominated so that electrons/positrons in the magnetar wind are accelerated by a diffusive shock. However, theoretical modeling of pulsar wind nebulae shows that in many cases the magnetic field energy in the pulsar wind may be strong enough to suppress diffusive shock acceleration. In this paper, we investigate the reverse shock emission and the forward shock emission with an arbitrary magnetization parameter σ of a magnetar wind. We find that the reverse shock emission strongly depends on σ, and in particular that σ ~ 0.3 leads to the strongest reverse shock emission. Future observations would be helpful to diagnose the composition of the magnetar wind.

  17. Monte Carlo simulation for thermal assisted reversal process of micro-magnetic torus ring with bistable closure domain structure

    NASA Astrophysics Data System (ADS)

    Terashima, Kenichi; Suzuki, Kenji; Yamaguchi, Katsuhiko

    2016-04-01

    Monte Carlo simulations were performed for temperature dependences of closure domain parameter for a magnetic micro-torus ring cluster under magnetic field on limited temperature regions. Simulation results show that magnetic field on tiny limited temperature region can reverse magnetic closure domain structures when the magnetic field is applied at a threshold temperature corresponding to intensity of applied magnetic field. This is one of thermally assisted switching phenomena through a self-organization process. The results show the way to find non-wasteful pairs between intensity of magnetic field and temperature region for reversing closure domain structure by temperature dependence of the fluctuation of closure domain parameter. Monte Carlo method for this simulation is very valuable to optimize the design of thermally assisted switching devices.

  18. Polarity Reversal of the Solar Photospheric Magnetic Field During Activity Cycle 24

    NASA Astrophysics Data System (ADS)

    Sun, Xudong; Hoeksema, Jon Todd; Liu, Yang; Zhao, Junwei

    2014-06-01

    The large-scale solar magnetic field reverses its polarity during the maximum phase of each activity cycle. As observed on the photosphere, active region (AR) magnetic flux migrates poleward in narrow, sheared streams resulted from large-scale flows and diffusion. A small net flux of the trailing sunspot polarity eventually aggregates at high latitudes, manifesting the poloidal field of the next cycle. We characterize this process for the ongoing cycle 24 based on four years' line-of-sight magnetograms from the Helioseismic and Magnetic Imager (HMI). The axial dipole component reversed sign in early 2012, but the poleward flux migration was grossly out of phase in the two hemispheres. As a proxy, the northern polar field (taken as mean above 70 degrees latitude) switched from negative to positive in late 2012, whereas the southern remained positive as of March 2014. Three factors that are in line with the surface flux transport model may have contributed. First, AR emergence started and peaked earlier in the north. Second, several ARs with small or inverse tilt angles (w.r.t. the Joy's law) emerged in the south in late 2010. Third, meridional flow speed inferred from helioseismology varied greatly prior to 2013; slower streams (compared to a three-year mean at the same latitude) appeared earlier in the north. We correlate HMI with the long-running Wilcox Solar Observatory (WSO) dataset, and compare the current cycle with the previous three.

  19. Magnetization reversal in individual cobalt micro- and nanowires grown by focused-electron-beam-induced-deposition.

    PubMed

    Fernández-Pacheco, A; De Teresa, J M; Szkudlarek, A; Córdoba, R; Ibarra, M R; Petit, D; O'Brien, L; Zeng, H T; Lewis, E R; Read, D E; Cowburn, R P

    2009-11-25

    We systematically study individual micro- and nanometric polycrystalline cobalt wires grown by focused-electron-beam-induced-deposition. The deposits were grown in a range of aspect ratios varying from 1 up to 26. The minimum lateral dimension of the nanowires was 150 nm, for a thickness of 40 nm. Atomic force microscopy images show beam-current-dependent profiles, associated with different regimes of deposition. The magnetization reversal of individual nanowires is studied by means of the spatially resolved magneto-optical Kerr effect. Abrupt switching is observed, with a systematic dependence on the wire's dimensions. This dependence of the coercive field is understood in magnetostatic terms, and agrees well with previous results on cobalt wires grown with different techniques. The influence of compositional gradients along the structural profile on the magnetic reversal is studied by using micromagnetic simulations. This work demonstrates the feasibility of using this technique to fabricate highly pure magnetic nanostructures, and highlights the advantages and disadvantages of the technique with respect to more conventional ones.

  20. Magnetic colloid by PLA: Optical, magnetic and thermal transport properties

    NASA Astrophysics Data System (ADS)

    Pandey, B. K.; Shahi, A. K.; Gopal, Ram

    2015-08-01

    Ferrofluids of cobalt and cobalt oxide nanoparticles (NPs) have been successfully synthesized using liquid phase-pulse laser ablation (LP-PLA) in ethanol and double distilled water, respectively. The mechanism of laser ablation in liquid media and formation process for Co target in double distilled water (DDW) and ethanol are speculated based on the reactions between laser generated highly nascent cobalt species and vaporized solvent media in a confined high temperature and pressure at the plume-surrounding liquid interface region. Optical absorption, emission, vibrational and rotational properties have been investigated using UV-vis absorption, photoluminescence (PL) and Fourier transform-infra red (FT-IR) spectroscopy, respectively. In this study optical band gap of cobalt oxide ferrofluids has been engineered using different pulse energy of Nd:YAG laser in the range of (2.80-3.60 eV). Vibrating sample magnetometer (VSM) is employed to determine the magnetic properties of ferrofluids of cobalt and cobalt oxide NPs while their thermal conductivities are examined using rotating disc method. Ferrofluids have gained enormous curiosity due to many technological applications, i.e. drug delivery, coolant and heating purposes.

  1. Surface-imprinted magnetic particles for highly selective sulfonamides recognition prepared by reversible addition fragmentation chain transfer polymerization.

    PubMed

    Xie, Xiaoyu; Liu, Xia; Pan, Xiaoyan; Chen, Liang; Wang, Sicen

    2016-01-01

    In this work, novel magnetic molecularly imprinted polymers (MMIPs) were prepared by reversible addition fragmentation chain transfer (RAFT) polymerization using sulfamerazine as the template. With the controlled/living property of RAFT polymerization, the resulting MMIPs showed high selectivity for sulfonamides recognition. The MMIPs were characterized by transmission electron microscopy, Fourier transform infrared, vibrating sample magnetometer, X-ray diffraction, X-ray photoelectron spectroscopy, and thermogravimetric analysis. The static and selectivity binding experiments demonstrated the desirable adsorption capacity and high selectivity of the MMIPs. The developed MMIPs were used as the solid-phase extraction sorbents to selectively extract four sulfonamides from aqueous solution. The recoveries of the spiked pond water ranged from 61.2 to 94.1% with RSD lower than 6.5%. This work demonstrated a versatile approach for the preparation of well-constructed MMIPs for application in the field of solid-phase extraction. PMID:26637219

  2. Plasma edge transport with magnetic islands—a comparison between tokamak and reversed-field pinch

    NASA Astrophysics Data System (ADS)

    Ciaccio, G.; Schmitz, O.; Abdullaev, S. S.; Frerichs, H.; Agostini, M.; Scarin, P.; Spizzo, G.; Vianello, N.; White, R. B.

    2014-06-01

    In the reversed-field pinch (RFP) edge, measured transport and flows are strongly influenced by magnetic islands (Vianello 2013 Nucl. Fusion 53 073025). In fact, these islands determine a differential radial diffusion of electrons and ions which, interacting with the wall, give rise to a characteristic edge ambipolar potential. Such island structures also arise in tokamak plasmas, when resonant magnetic perturbations (RMPs) are applied for control of edge-localized modes. They impose a characteristic modulation to edge electron density and temperature fields, in close correlation with the local magnetic vacuum topology (Schmitz 2012 Nucl. Fusion 52 054001). In order to develop a generic picture of particle transport with magnetic islands located in the plasma edge between RFPs and tokamaks with RMP, test-particle transport simulations are done on TEXTOR with the same tool used in RFX-mod, namely, the guiding-centre code ORBIT (White and Chance 1984 Phys. Fluids 27 2455-67). A typical TEXTOR discharge in the (m, n) = (12, 4) configuration is reconstructed and analysed with ORBIT. We use Poincaré and connection length analysis of electrons and ion orbits to analyse the magnetic structure taking into account the different gyro-orbits of both constituents. Density distributions of test ions and electrons are calculated and used to obtain an initial estimate of the plasma potential and radial electric field around the island.

  3. Effects Of Hydrothermal Alteration On Magnetic Properties And Magnetic Signatures - Implications For Predictive Magnetic Exploration Models

    NASA Astrophysics Data System (ADS)

    Clark, D.

    2012-12-01

    Magnetics is the most widely used geophysical method in hard rock exploration and magnetic surveys are an integral part of exploration programs for many types of mineral deposit, including porphyry Cu, intrusive-related gold, volcanic-hosted epithermal Au, IOCG, VMS, and Ni sulfide deposits. However, the magnetic signatures of ore deposits and their associated mineralized systems are extremely variable and exploration that is based simply on searching for signatures that resemble those of known deposits and systems is rarely successful. Predictive magnetic exploration models are based upon well-established geological models, combined with magnetic property measurements and geological information from well-studied deposits, and guided by magnetic petrological understanding of the processes that create, destroy and modify magnetic minerals in rocks. These models are designed to guide exploration by predicting magnetic signatures that are appropriate to specific geological settings, taking into account factors such as tectonic province; protolith composition; post-formation tilting/faulting/ burial/ exhumation and partial erosion; and metamorphism. Patterns of zoned hydrothermal alteration are important indicators of potentially mineralized systems and, if properly interpreted, can provided vectors to ore. Magnetic signatures associated with these patterns at a range of scales can provide valuable information on prospectivity and can guide drilling, provided they are correctly interpreted in geological terms. This presentation reviews effects of the important types of hydrothermal alteration on magnetic properties within mineralized systems, with particular reference to porphyry copper and IOCG deposits. For example, an unmodified gold-rich porphyry copper system, emplaced into mafic-intermediate volcanic host rocks (such as Bajo de la Alumbrera, Argentina) exhibits an inner potassic zone that is strongly mineralized and magnetite-rich, which is surrounded by an outer

  4. Reversible electrically-driven magnetic domain wall rotation in multiferroic heterostructures to manipulate suspended on-chip magnetic particles

    NASA Astrophysics Data System (ADS)

    Nowakowski, Mark; Sohn, Hyunmin; Liang, Cheng-Yen; Hockel, Joshua; Wetzlar, Kyle; Keller, Scott; McLellan, Brenda; Marcus, Matthew; Doran, Andrew; Young, Anthony; Kläui, Mathias; Carman, Gregory; Bokor, Jeffrey; Candler, Robert

    2015-03-01

    We experimentally demonstrate reversible electrically-driven, strain-mediated domain wall (DW) rotation in Ni rings fabricated on piezoelectric [Pb(Mg1/3Nb2/3) O3]0.66-[PbTiO3]0.34 (PMN-PT) substrates. An electric field applied across the PMN-PT substrate induces a strain in the Ni rings producing DW rotation around the ring toward the dominant PMN-PT strain axis by inverse magnetostriction. We observe DWs reversibly cycled between their initial and rotated state as a function of the applied electric field with x-ray magnetic circular dichroism photo-emission electron microscopy. The DW rotation is analytically predicted using a fully coupled micromagnetic/elastodyanmic multi-physics simulation to verify that the experimental behavior is caused by the electrically-generated strain in this multiferroic system. Finally, this DW rotation is used to capture and manipulate magnetic particles in a fluidic environment to demonstrate a proof-of-concept energy-efficient pathway for multiferroic-based lab-on-a-chip applications. Supported by TANMS (NSF 11-537), E3S, US Dept of Energy (DE-AC02-05CH11231), EU, and DFG.

  5. Nature of magnetization reversal in exchange-coupled polycrystalline NiO-Co bilayers

    NASA Astrophysics Data System (ADS)

    Chopra, Harsh Deep; Yang, David X.; Chen, P. J.; Brown, H. J.; Swartzendruber, L. J.; Egelhoff, W. F.

    2000-06-01

    The nature of magnetization reversal in exchange-coupled NiO-Co polycrystalline bilayers was investigated. As-deposited bilayers exhibit a moderate value of exchange bias HE (=-0.9 mT) and a significantly enhanced coercivity (HNiO-Coc=12.4 mT), which is roughly 5 times the coercivity of a reference Co single film (HCoc=2.7 mT). Real time investigation of magnetization reversal in exchange-coupled NiO-Co bilayers shows that reversal is highly local and nonuniform in nature. It is preceded by the formation of precursors or embryos of reversed domains as the applied field reaches a critical value ≅8.8-9.0 mT. Once this critical applied field value is reached, numerous reversed domains are formed. Growths of such reversed domains occur primarily by the abrupt nucleation and the subsequent coalescence together of reversed domains; wall motion is not the dominant growth mode. Clear evidence is presented which shows that the strength of exchange bias varies at the microscopic scale across the sample. This manifests itself as different microscopic regions switching abruptly at different fields, and a given microscopic area switching at different fields in the positive and negative field directions. When the applied field is along the unidirectional anisotropy, reversal of a given strongly coupled microscopic region is aided by exchange bias, and such a region switches first; the same region undergoes reversal last when the polarity of the applied field is changed to oppose unidirectional anisotropy. Significantly, it was found that, locally, the measured value of exchange bias may vary by a factor of 3 or more from the macroscopically measured value of HE (=-0.9 mT) obtained from the shift of the M-H loop. High-resolution transmission electron microscopy (HRTEM) shows that that the local variation in HE may be explained by considering the underlying microstructure and interfacial topography of the NiO-Co interface. HRTEM results show that the NiO surface parallel to the

  6. Reversible and Nonvolatile Modulations of Magnetization Switching Characteristic and Domain Configuration in L10-FePt Films via Nonelectrically Controlled Strain Engineering.

    PubMed

    Feng, Chun; Zhao, Jiancheng; Yang, Feng; Hao, Shijie; Gong, Kui; Hu, Di; Cao, Yi; Jiang, Xumin; Wang, Zhongqiang; Chen, Lei; Li, Sirui; Sun, Li; Cui, Lishan; Yu, Guanghua

    2016-03-23

    Reversible and nonvolatile modulation of magnetization switching characteristic in ferromagnetic materials is crucial in developing spintronic devices with low power consumption. It is recently discovered that strain engineering can be an active and effective approach in tuning the magnetic/transport properties of thin films. The primary method in strain modulation is via the converse piezoelectric effect of ferroelectrics, which is usually volatile due to the reliance of the required electric field. Also the maximum amount of deformation in ferroelectrics is usually limited to be less than 1%, and the corresponding magnetoelastic strain energy introduced to ferromagnetic films is on the order of 10(4) J/m(3), not enough to overcome magnetocrystalline anisotropy energy (Ku) in many materials. Different from using conventional strain inducing substrates, this paper reports on the significantly large, reversible, and nonvolatile lattice strain in the L10-FePt films (up to 2.18%) using nonelectrically controlled shape memory alloy substrates. Introduced lattice strain can be large enough to effectively affect domain structure and magnetic reversal in FePt. A noticeable decrease of coercivity field by 80% is observed. Moreover, the coercivity field tunability using such substrates is nonvolatile at room temperature and is also reversible due to the characteristics of the shape memory effect. This finding provides an efficient avenue for developing strain assisted spintronic devices such as logic memory device, magnetoresistive random-access memory, and memristor.

  7. Time-Reversal Symmetry Breaking and Consequent Physical Responses Induced by All-In-All-Out Type Magnetic Order on the Pyrochlore Lattice

    NASA Astrophysics Data System (ADS)

    Arima, Taka-Hisa

    2014-03-01

    Pyrochlore-type 5d transition-metal oxide compounds Cd2Os2O7 and R2Ir2O7 (R =rare earth) undergo a metal-insulator transition accompanied by a magnetic transition. Recently, the magnetic structures of Cd2Os2O7 and Eu2Ir2O7 were investigated by means of resonant x-ray magnetic scattering. The x-ray data indicated the all-in/all-out type magnetic order. The all-in/all-out order breaks the time-reversal symmetry, while the spontaneous magnetization is essentially absent. The magnetic order can be viewed as ferroic magnetic octupolar order. The magnetic order is expected to provide several unique physical properties like quadratic magnetization. linear magneto-capacitance, linear magneto-resistance, linear magneto-mechanical coupling and so on. The symmetry breaking results in two non-equivalent domains, ``all-in/all-out'' and ``all-out/all-in.'' Interestingly, some theoretical works predict that a peculiar metallic state would appear on the domain wall. The observation and control of the domain distribution are essential for studying verious exotic physical responses. We have developed an x-ray technique for domain imaging and started studying the effects of external stimuli on the domain distribution. This work was performed in collaboration with S. Tardif, S. Takeshita, H. Ohsumi, D. Uematsu, H. Sagayama, J. J. Ishikawa, S. Nakatsuji, J. Yamaura, and Z. Hiroi.

  8. Microstructure and Magnetic Properties of Electrodeposited Cobalt Film

    SciTech Connect

    Bhuiyan, Md S; Taylor, B. J.; Paranthaman, Mariappan Parans; Thompson, James R; Sinclair, J.

    2008-01-01

    Cobalt films were electrodeposited onto both iron and copper substrates from an aqueous solution containing a mixture of cobalt sulfate, boric acid, sodium citrate, and vanadyl sulfate. The structural, intermetallic diffusion and magnetic properties of the electrodeposited films were studied. Cobalt electrodeposition was carried out in a passively divided cell aided by addition of vanadyl sulfate to keep the counter electrode clean. The divided electrolytic cell with very negative current densities cause the electrodeposited Co to adopt a face-centered cubic (fcc) structure, which is more magnetically reversible than the hexagonally close-packed (hcp) structured Co. The coercive field is also significantly less in the fcc-electrodeposited cobalt than in the hcp. SEM images show dense, uniform Co films without any cracks or porosity. Beside the deposition current, thickness of the film was also found to affect the crystal orientation particularly on iron substrates. Diffusion of cobalt film into the iron substrate was studied under reduced environment and a fast process was observed.

  9. Electronic and Magnetic Properties of Silicene and Silicane Nanoribbons

    NASA Astrophysics Data System (ADS)

    Li, Kai; Lee, Anna Shin Hwa; Zhang, Yong-Wei; Pan, Hui

    2013-06-01

    In this paper, first-principles calculations are carried out to study the electronic and magnetic properties of silicene and silicane nanoribbons, with and without H-passivation at the edges. We predict that the armchair nanoribbons are nonmagnetic and semiconducting. Interestingly, the band gaps of armchair silicene nanoribbons show oscillating behavior as the ribbon width increases. When their edges are passivated with H atoms, However, the oscillating phase is reversed. The zigzag nanoribbons are anti-ferromagnetic and semiconducting in their ground states, except that the zigzag silicane nanoribbons with edges passivated by H atoms are nonmagnetic. The zigzag silicane nanoribbons with bare edges show the highest magnetic moments in their ground states. The band gaps of zigzag nanoribbons in their ground states decrease with the increment of width. The metastable states of zigzag silicene nanoribbons are ferromagnetic and metallic. The zigzag silicane nanoribbons with bare edges are ferromagnetic and semiconducting in their metastable states. The silicene/silicane nanoribbons with attractive functions, which are achievable by edge engineering or external fields, may be applied to spintronic technologies and nanodevices.

  10. Brunhes-Matuyama Magnetic Polarity Reversal Tracing using Chinese loess10Be

    NASA Astrophysics Data System (ADS)

    Zhou, W.; Beck, W.; Kong, X.; An, Z.; Qiang, X.; Wu, Z.; Xian, F.; Ao, H.

    2014-12-01

    The geomagnetic polarity reversal is generally considered to occur synchronously around the world, and is commonly used as a time marker. However, in the case of the most recent reversal, the Brunhes-Matuyama (B-M) reversal (~780 ka), comparison of paleomagnetic studies in Chinese loess-paleosol sequences versus marine sediments revealed a marked discrepancy in timing of this event (Tauxe et al., 1996; Zhou and Shackleton, 1999), leading to the debate on uncertainties of paleoclimatic correlation between the Chinese loess-paleosol sequences and marine sediments (Wang et al., 2006; Liu et al., 2008; Jin and Liu, 2011). Based on this issue, here we propose to use the cosmogenic 10Be to address this conundrum. 10Be is a long-lived radionuclide produced in the atmosphere by cosmic ray spallation reactions and carried to the ground attached to aerosols. Its atmospheric production rate is inversely proportional to the geomagnetic field intensity (Masarik and Beer, 1999). This allows us to reconstruct past geomagnetic field intensity variations using 10Be concentrations recorded in different sedimentary archives. We carried out the 10Be studies in Luochuan and Xifeng sections in Chinese Loess Plateau, both loess profiles show that 10Be production rate was at a maximum-an indication of the dipole field reversal-at ca. 780 ± 3 ka BP., in paleosol unit S7corresponding to MIS 19. These results have proven that the timing of B-M reversal recorded in Chinese loess is synchronous with that seen in marine records (Tauxe et al., 1996) and reaffirmed the conventional paleoclimatic correlation of loess-paleosol sequences with marine isotope stages and the standard loess timescale as correct. However, it is ~25 ka younger than the age (depth) of the magnetic polarity reversal recorded in these same Chinese loess-paleosol sequences, demonstrating that loess magnetic overprinting has occurred. 1.Jin, C.S.,et al., 2011,PALAEOGEOGR PALAEOCL, 299, 309-3172.Liu, Q.S., et al., 2008, EARTH

  11. Tin dioxide nanoparticles: Reverse micellar synthesis and gas sensing properties

    SciTech Connect

    Ahmed, Jahangeer; Vaidya, Sonalika; Ahmad, Tokeer; Sujatha Devi, P.; Das, Dipankar; Ganguli, Ashok K.

    2008-02-05

    Tin dioxide (SnO{sub 2}) nanoparticles have been synthesized by reverse micellar route using cetyltrimethyl ammoniumbromide (CTAB) as the surfactant. Monophasic tin dioxide (SnO{sub 2}) was obtained using NaOH as the precipitation agent at 60 deg. C, however, when liquor NH{sub 3} was used as precipitating agent then crystalline SnO{sub 2} nanoparticles are obtained at 500 deg. C. SnO{sub 2} prepared using NaOH show crystallite size of 4 and 12 nm after heating at 60 and 500 deg. C respectively using X-ray line broadening studies. Transmission electron microscopy (TEM) studies show agglomerated particles of sizes 70 and 150 nm, respectively. The grain size was found to be 6-8 nm after heating the precursor obtained (using liquor NH{sub 3}) at 500 deg. C by X-ray line broadening and the TEM studies. Dynamic light-scattering (DLS) studies show the aggregates of SnO{sub 2} nanoparticles with uniform size distribution. Moessbauer studies show an increase of s-electron density at the Sn sites compared to bulk SnO{sub 2} and a finite quadrupole splitting indicative of lowering of symmetry around tin atoms. The gas sensing characteristics have also been investigated using n-butane which show high sensitivity and fast recovery time.

  12. Magnetic properties of the magnetophotonic crystal based on bismuth iron garnet

    NASA Astrophysics Data System (ADS)

    Popova, Elena; Magdenko, Liubov; Niedoba, Halina; Deb, Marwan; Dagens, Béatrice; Berini, Bruno; Vanwolleghem, Mathias; Vilar, Christèle; Gendron, François; Fouchet, Arnaud; Scola, Joseph; Dumont, Yves; Guyot, Marcel; Keller, Niels

    2012-11-01

    This article reports on the magnetism of continuous and patterned bismuth iron garnet (Bi3Fe5O12 or BIG) thin films for magnetophotonic crystal (MPC) applications. The exact knowledge of the magnetic properties is crucial for the design of fully functional MPC. BIG thin films were grown on several types of isostructural substrates by pulsed laser deposition. The growth conditions and bismuth transfer were optimized to obtain good quality magneto-optically active films compatible with nanostructuring process. MPC were successfully fabricated from BIG/GGG(001) films with low roughness and high Faraday rotation. Magnetic characteristics (magnetization, anisotropy, magnetic domains, magnetization reversal) of the continuous BIG films and MPC were extensively studied and compared to the results of the micromagnetic simulations performed for MPC with different anisotropy. The present study shows that the fabrication of the MPC structure lowers the magnetocrystalline and uniaxial in-plane anisotropies and induces a partial out-of-plane magnetization. External field smaller than 2000 G is sufficient to ensure the out-of-plane saturation of magnetization for optimum device operation, in agreement with micromagnetic calculations. The experimentally determined magnetic properties of MPC are fully compatible with the device operation.

  13. Kagome network compounds and their novel magnetic properties.

    PubMed

    Pati, Swapan K; Rao, C N R

    2008-10-21

    Compounds possessing the Kagome network are truly interesting because of their unusual low-energy properties. They exhibit magnetic frustration because of the triangular lattice inherent to the hexagonal bronze structure they possess, as indeed demonstrated by some of the Fe(3+) jarosites, but this is not the general case. Kagome compounds formed by transition metal ions with varying spins exhibit novel magnetic properties, some even showing evidence for magnetic order and absence of frustration. We describe the structure and magnetic properties of this interesting class of materials and attempt to provide an explanation for the variety of properties on the basis of theoretical considerations.

  14. Reversible magnetic resonance imaging changes in a case of neuroleptic malignant syndrome.

    PubMed

    Jain, Rajendra Singh; Gupta, Pankaj Kumar; Gupta, Ishwar Dayal; Agrawal, Rakesh; Kumar, Sunil; Tejwani, Shankar

    2015-08-01

    Neuroleptic malignant syndrome (NMS) is a life-threatening neurologic emergency associated with the use of mainly typical antipsychotic drugs. It is characterized by fever, altered mental status, generalized rigidity, autonomic instability, myoclonus, raised creatine phosphokinase, rhabdomyolysis, and leukocytosis. Neuroimaging (brain computed tomography/magnetic resonance imaging [MRI]) is usually normal in most of the cases of NMS. Magnetic resonance imaging findings have not been well elucidated in NMS as yet. Very few cases have been reported worldwide. We herein, report a case of a 42-year-old patient of NMS, who presented to us with reversible changes in MRI brain. This case report highlights the possible MRI changes in NMS and their plausible mechanism. PMID:25769796

  15. Magnetic diagnostic suite of the C-2 field-reversed configuration experiment confinement vessela)

    NASA Astrophysics Data System (ADS)

    Thompson, M. C.; Douglass, J. D.; Feng, P.; Knapp, K.; Luo, Y.; Mendoza, R.; Patel, V.; Tuszewski, M.; Van Drie, A. D.

    2012-10-01

    Magnetic measurements are a fundamental part of determining the size and shape of field-reversed configuration (FRC) plasmas in the C-2 device. The magnetic probe suite consists of 44 in-vessel and ex-vessel probes constructed using various technologies: ultra-high vacuum compatible mineral-insulated cable, nested triple axis coils hand-wound on ceramic bobbins, and commercial chip inductors mounted on printed circuit boards. Together, these probes measure the three-dimensional excluded flux profile of the FRC, which approximates the shape of the separatrix between the confined plasma volume and the scrape-off layer. High accuracy is achieved by using the extensive probe measurements to compensate for non-ideal effects such as flux leakage through the vacuum vessel and bulk motion of the FRC towards the wall. A subset of the probes is also used as a set of Mirnov arrays that provide sensitive detection of perturbations and oscillations of the FRC.

  16. Analysis of antimycin A by reversed-phase liquid chromatography/nuclear magnetic-resonance spectrometry

    USGS Publications Warehouse

    Ha, Steven T.K.; Wilkins, Charles L.; Abidi, Sharon L.

    1989-01-01

    A mixture of closely related streptomyces fermentation products, antimycin A, Is separated, and the components are identified by using reversed-phase high-performance liquid chromatography with directly linked 400-MHz proton nuclear magnetic resonance detection. Analyses of mixtures of three amino acids, alanine, glycine, and valine, are used to determine optimal measurement conditions. Sensitivity increases of as much as a factor of 3 are achieved, at the expense of some loss in chromatographic resolution, by use of an 80-μL NMR cell, Instead of a smaller 14-μL cell. Analysis of the antimycin A mixture, using the optimal analytical high performance liquid chromatography/nuclear magnetic resonance conditions, reveals it to consist of at least 10 closely related components.

  17. Two-dimensional nonlinear cylindrical equilibria with reversed magnetic shear and sheared flow

    NASA Astrophysics Data System (ADS)

    Kuiroukidis, Ap; Throumoulopoulos, G. N.; Throumoulopoulos

    2014-02-01

    Nonlinear translational symmetric equilibria with up to quartic flux terms in free functions, reversed magnetic shear, and sheared flow are constructed in two ways: (i) quasi-analytically by an ansatz, which reduces the pertinent generalized Grad-Shafranov equation to a set of ordinary differential equations and algebraic constraints which is then solved numerically, and (ii) completely numerically by prescribing analytically a boundary having an X-point. This latter case presented in Sec. 4 is relevant to the International Thermonuclear Experimental Reactor project. The equilibrium characteristics are then examined by means of pressure, safety factor, current density, and electric field. For flows parallel to the magnetic field, the stability of the equilibria constructed is also examined by applying a sufficient condition. It turns out that the equilibrium nonlinearity has a stabilizing impact, which is slightly enhanced by the sheared flow. In addition, the results indicate that the stability is affected by the up-down asymmetry.

  18. Anomalous Beam-Ion Loss in TFTR Reversed Magnetic Shear Plasmas

    SciTech Connect

    Ruskov, E.; Bell, M.; Budny, R.V.; McCune, D.C.; Medley, S.S.; Redi, M.H.; Scott, S.; Synakowski, E.J.; von Goeler, S.; White, R.B.; Zweben, S.J.

    1999-02-01

    Anomalous beam-ion loss has been observed in an experiment with short tritium beam pulses injected into deuterium-beam-heated Tokamak Fusion Test Reactor plasmas (P{sub NBI}=15 thinspthinspMW) with reversed magnetic shear (RS). Comparisons of the measured total 14thinspthinspMeV neutron emission, the neutron flux along eight radial locations, and the perpendicular plasma stored energy with predictions from an extensive set of TRANSP simulations suggest that about 40{percent} beam power is lost on a time scale much shorter than the tritium beam pulse length {Delta}t=70 thinspthinspms. In contrast with recent results [K. Tobita {ital et al.,} Nucl.thinspthinspFusion {bold 37}, 1583 (1997)] from RS experiments at JT-60U, we were not able to show conclusively that magnetic field ripple is responsible for this anomaly. {copyright} {ital 1999} {ital The American Physical Society}

  19. Anomalous Beam-Ion Loss in TFTR Reversed Magnetic Shear Plasmas

    NASA Astrophysics Data System (ADS)

    Ruskov, E.; Bell, M.; Budny, R. V.; McCune, D. C.; Medley, S. S.; Redi, M. H.; Scott, S.; Synakowski, E. J.; von Goeler, S.; White, R. B.; Zweben, S. J.

    1999-02-01

    Anomalous beam-ion loss has been observed in an experiment with short tritium beam pulses injected into deuterium-beam-heated Tokamak Fusion Test Reactor plasmas ( PNBI = 15 MW) with reversed magnetic shear (RS). Comparisons of the measured total 14 MeV neutron emission, the neutron flux along eight radial locations, and the perpendicular plasma stored energy with predictions from an extensive set of TRANSP simulations suggest that about 40% beam power is lost on a time scale much shorter than the tritium beam pulse length Δt = 70 ms. In contrast with recent results [K. Tobita et al., Nucl. Fusion 37, 1583 (1997)] from RS experiments at JT-60U, we were not able to show conclusively that magnetic field ripple is responsible for this anomaly.

  20. Loess 10Be evidence for an asynchronous Brunhes-Matuyama magnetic polarity reversal

    NASA Astrophysics Data System (ADS)

    Zhou, Weijian; Beck, J. Warren; Kong, Xianghui; An, Zhisheng; Qiang, Xiaoke; Wu, Zhenkun; Xian, Feng; Ao, Hong

    2015-04-01

    In Chinese loess the Brunhes-Matuyama (B-M) geomagnetic reversal appears to occur about 25 ka prior to the established axial dipole reversal age found in many marine sediments, i.e., in Chinese loess this magnetic reversal boundary is found in glacial loess unit L8 which is thought to be correlated with Marine Isotope Stage 20 (MIS 20), in marine sediment records, however, this boundary is commonly found in interglacial period of MIS 19 (Tauxe et al., 1996; Zhou and Shackleton, 1999), leading to the debate on uncertainties of paleoclimatic correlation between the Chinese loess-paleosol sequences and marine sediments (Wang et al., 2006; Liu et al., 2008; Jin and Liu, 2011). Based on this issue, here we propose to use the cosmogenic 10Be to address this conundrum. 10Be is a long-lived radionuclide produced in the atmosphere by cosmic ray spallation reactions and carried to the ground attached to aerosols. Its atmospheric production rate is inversely proportional to the geomagnetic field intensity (Masarik and Beer, 1999). This allows us to reconstruct past geomagnetic field intensity variations using 10Be concentrations recorded in different sedimentary archives. We carried out both the 10Be studies and paleogeomagnetic measurements in Luochuan and Xifeng sections in Chinese Loess Plateau. Both loess profiles show that 10Be production rate was at a maximum-an indication of the dipole field reversal-at ca. 780 ± 3 ka BP., in paleosol unit S7 corresponding to MIS 19, proving that the timing of B-M reversal recorded in Chinese loess is synchronous with that seen in marine records (Tauxe et al., 1996). These results reaffirmed the conventional paleoclimatic correlation of loess-paleosol sequences with marine isotope stages and the standard loess timescale as correct. However, it is ~25 ka younger than the age (depth) of the paleogeomagnetic measurements which show that the B-M boundary is in L8 in these two Chinese loess-paleosol sequences, demonstrating that loess

  1. Reversible “triple-Q” elastic field structures in a chiral magnet

    PubMed Central

    Hu, Yangfan; Wang, Biao

    2016-01-01

    The analytical solution of the periodic elastic fields in chiral magnets caused by presence of periodically distributed eigenstrains is obtained. For the skyrmion phase, both the periodic displacement field and the stress field are composed of three “triple-Q” structures with different wave numbers. The periodic displacement field, obtained by combining the three “triple-Q” displacement structures, is found to have the same lattice vectors with the magnetic skyrmion lattice. We find that for increasing external magnetic field, one type of “triple-Q” displacement structure and stress structure undergo a “configurational reversal”, where the initial and the final field configuration share similar pattern but with opposite direction of all the field vectors. The solution obtained is of fundamental significance for understanding the emergent mechanical properties of skyrmions in chiral magnets. PMID:27457629

  2. Direct imaging of the magnetic polarity and reversal mechanism in individual Fe(3-x)O4 nanoparticles.

    PubMed

    Moya, Carlos; Iglesias-Freire, Óscar; Pérez, Nicolás; Batlle, Xavier; Labarta, Amilcar; Asenjo, Agustina

    2015-05-01

    This work reports on the experimental characterization of the magnetic domain configurations in cubic, isolated Fe3-xO4 nanoparticles with a lateral size of 25-30 nm. The magnetic polarity at remanence of single domain ferrimagnetic Fe3-xO4 nanoparticles deposited onto a carbon-silicon wafer is observed by magnetic force microscopy. The orientations of these domains provide a direct observation of the magneto-crystalline easy axes in each individual nanoparticle. Furthermore, the change in the domain orientation with an external magnetic field gives evidence of particle magnetization reversal mediated by a coherent rotation process that is also theoretically predicted by micromagnetic calculations.

  3. Variation of Magnetic Fluctuation due to Gas Puffing in Edge Region of Reversed-Field Pinch Plasma

    NASA Astrophysics Data System (ADS)

    Yambe, Kiyoyuki; Hirano, Yoichi; Sakakita, Hajime; Koguchi, Haruhisa

    2016-09-01

    We measured the variation of magnetic and electrostatic fluctuations observed during the gas puffing in the edge region of the toroidal pinch experiment-reversed experiment (TPE-RX) reversed-field pinch plasma. In the short period in which the electron density increased slowly just after the gas puffing, the confinement of fast electrons in the core region was maintained by the decrease in the fast radial magnetic fluctuation with the deepening of the reversal of the toroidal field. During the following period in which the electron density increased rapidly, the radial gradient of electron density decreased, and the loss of fast electrons from the core region increased owing to the increase in the toroidal and radial magnetic fluctuations in the high-frequency band, although the poloidal magnetic fluctuation decreased. Therefore, the confinement of fast electrons would be maintained by keeping the radial gradient of plasma thermal pressure with a moderate neutral particle supply of small quantity in a short time.

  4. Helical states with ordered magnetic topology in the Reversed Field Pinch

    NASA Astrophysics Data System (ADS)

    Bonfiglio, D.; Cappello, S.; Gobbin, M.; Spizzo, G.

    2008-11-01

    The reversed field pinch (RFP) configuration for magnetic confinement has shown to develop helical configurations characterized by good magnetic surfaces both in experiments and visco-resistive 3D MHD numerical computations [1]. In the RFX-mod experiment, quasi-single helicity (QSH) states with ordered magnetic topology have been found to develop both spontaneously during high current discharges [2] and in a stimulated way through the periodic oscillation of the toroidal flux (so-called OPCD technique) [3]. In both cases, the expulsion of the separatrix of the dominant mode has proved to be the key for significant chaos healing [4], as expected by theory [5]. In this work, we present results of visco-resistive 3D MHD numerical modeling aiming at clarifying the mechanism and the conditions for separatrix expulsion and chaos healing in spontaneous and stimulated cases. The effect is investigated by reconstruction of the magnetic topology through field line tracing algorithms and by study of test particle dynamics. [1] S. Cappello, Plasma Phys. Control. Fusion 46, B313 (2004) & references therein. [2] M. Valisa et al., invited oral, EPS Conf. on Plasma Physics (2008). [3] D. Terranova et al., Phys. Rev. Lett. 99, 095001 (2007). [4] R. Lorenzini et al., Phys. Rev. Lett. 101, 025005 (2008). [5] D. F. Escande, R. Paccagnella et al., Phys. Rev. Lett. 85, 3169 (2000).

  5. Chitosan-Coated Magnetic Nanoparticles Prepared in One Step by Reverse Microemulsion Precipitation

    PubMed Central

    López, Raúl G.; Pineda, María G.; Hurtado, Gilberto; de León, Ramón Díaz; Fernández, Salvador; Saade, Hened; Bueno, Darío

    2013-01-01

    Chitosan-coated magnetic nanoparticles (CMNP) were obtained at 70 °C and 80 °C in a one-step method, which comprises precipitation in reverse microemulsion in the presence of low chitosan concentration in the aqueous phase. X-ray diffractometry showed that CMNP obtained at both temperatures contain a mixture of magnetite and maghemite nanoparticles with ≈4.5 nm in average diameter, determined by electron microscopy, which suggests that precipitation temperature does not affect the particle size. The chitosan coating on nanoparticles was inferred from Fourier transform infrared spectrometry measurements; furthermore, the carbon concentration in the nanoparticles allowed an estimation of chitosan content in CMNP of 6%–7%. CMNP exhibit a superparamagnetic behavior with relatively high final magnetization values (≈49–53 emu/g) at 20 kOe and room temperature, probably due to a higher magnetite content in the mixture of magnetic nanoparticles. In addition, a slight direct effect of precipitation temperature on magnetization was identified, which was ascribed to a possible higher degree of nanoparticles crystallinity as temperature at which they are obtained increases. Tested for Pb2+ removal from a Pb(NO3)2 aqueous solution, CMNP showed a recovery efficacy of 100%, which makes them attractive for using in heavy metals ion removal from waste water. PMID:24084716

  6. Magnetization reversal in the orthochromite Y0 . 5 Gd0.5 CrO3

    NASA Astrophysics Data System (ADS)

    Duran, Alejandro; Escudero, Roberto; Escamilla, Raul; Morales, Fransisco; Verdin, Eduardo

    Complex oxide of transition metal with perovskite structure represent fascinating playground for basic solid state research: new electronics and exotic ground states emerge via the competing interplay like spin, orbital, charge as well as lattice degree of freedom. Accordingly, orthochromites are not exception to the rule. In these compounds have been found ferroelectric polarization, spin reorientation transition along with the characteristic behavior known as; magnetization reversal (MR) consisting that a characteristic temperature, T*, the system becomes diamagnetic. In this work, the magnetic behavior of the equimolar Y0.5Gd0.5CrO3 composition was studied. Negative magnetization was observed at T*~70 K in FC mode, and applied field of 100 Oe. The characteristic hysteresis loop in the M-H graph of the pristine sample disappears for a wide range of temperature below of TN, and the characteristic spin reorientation is shifted from 14 K in GdCrO3 to 5 K for Y0.5Gd0.5CrO3. The negative magnetization is explained according the model that take into account the anisotropic and antisymmetric exchange interaction between Gd +3 - Cr +3 sublattice. A.D. and R.E. thanks to grants by DGAPA-PAPIIT, IN103213 and IN 106014 respectively.

  7. Probe measurements of the three-dimensional magnetic field structure in a rotating magnetic field sustained field-reversed configuration

    SciTech Connect

    Velas, K. M.; Milroy, R. D.

    2014-01-15

    A translatable three-axis probe was constructed and installed on the translation, confinement, and sustainment upgrade (TCSU) experiment. With ninety windings, the probe can simultaneously measure B{sub r}, B{sub θ}, and B{sub z} at 30 radial positions, and can be placed at any desired axial position within the field reversed configuration (FRC) confinement chamber. Positioning the probe at multiple axial positions and taking multiple repeatable shots allows for a full r-z map of the magnetic field. Measurements were made for odd-parity rotating magnetic field (RMF) antennas and even-parity RMF. The steady state data from applying a 10 kHz low pass filter used in conjunction with data at the RMF frequency yields a map of the full 3D rotating field structure. Comparisons will be made to the 3D magnetic structure predicted by NIMROD simulations, with parameters adjusted to match that of the TCSU experiments. The probe provides sufficient data to utilize a Maxwell stress tensor approach to directly measure the torque applied to the FRC's electrons, which combined with a resistive torque model, yields an estimate of the average FRC resistivity.

  8. Reverse Polarity Magnetized Melt Rocks from the Cretaceous/Tertiary Chicxulub Structure, Yucatan Peninsula, Mexico

    NASA Technical Reports Server (NTRS)

    Urrutia-Fucugauchi, J.; Marin, Luis; Sharpton, Virgil L.

    1994-01-01

    We report paleomagnetic results for core samples of the breccia and andesitic rocks recovered from the Yucatan-6 Petrolcos Mexicanos exploratory well within the Chicxulub structure (about 60 km SSW from its center), northern Yucatan, Mexico. A previous study has shown that the rocks studied contain high iridium levels and shocked breccia clasts and an Ar/Ar date of 65.2 +/- 0.4 Ma. Andesitic rocks are characterized by stable single-component magnetizations with a mean inclination of -42.6 deg +/- 2.4 deg. Breccias present a complex paleomagnetic record characterized by multivectorial magnetizations with widely different initial NRM inclinations. However, after alternating field demagnetization, well defined characteristic components with upward inclinations are defined. IRM acquisition experiments, comparison of IRM and NRM coercivity spectra and the single component magnetization of the andesitic rocks indicate the occurrence of iron-rich titanomagnetites of single or pseudo-single domain states as the dominant magnetic carriers. Mean inclinations from the andesitic rocks and most of the breccia samples give a mean inclination of about -40 deg to -45 deg, indicating a reverse polarity for the characteristic magnetization that is consistent with geomagnetic chron 29R, which spans the Cretaceous/Tertiary (K/T) boundary. The inclination is also consistent with the expected value (and corresponding paleolatitude) for the site estimated from the reference polar wander curve for North America. We suggest that the characteristic magnetizations for the andesitic and breccia rocks are the result of shock heating at the time of formation of the impact structure and that the age, polarity and pateolatitude are consistent with a time at the K/T boundary.

  9. Synthesis and Properties of Magnetic Fine Particles

    NASA Astrophysics Data System (ADS)

    Tang, Zhongxun

    Magnetic fine particles with a variety of compositions and sizes have been prepared by aerosol and coprecipitation technique. Their magnetic properties are shown to be either similar to or quite different from those of their bulk counterparts. Iron oxide, barium iron oxide and neodynium iron based fine particles have been synthesized by an aerosol technique which produced particles with average size of about 100 nm. It was found that the as-received samples were usually in thermally unstable states because of their short residence time (seconds) at the high temperature when they were created. Heat treatment turned these as -received particles into more stable phases. The final product depended on temperature, environment and composition of the initial solution. Cation and anion effects and solvent effects on the formation and morphology of the final particle have been also observed. Manganese ferrite fine particles have been made by hydroxide induced coprecipitation of mixed iron and manganese salt solutions. The particle size appeared to be an unique function of the ratio of the metallic ion concentration to the hydroxide ion concentration when the digestion conditions were fixed. The system which used ferric salt created small MnFe_2 O_4 particles with size controllable between 5 and 25 nm. The digestion process could be described by an Ostwald ripening in which OH^- acts as a catalyst. Variation of cations showed that their oxidation states had a strong influence on the particle size. The system which used ferrous salt, however, produced larger ferrite particles (above 50 nm) with single ferrite phase (Mn_ xFe_{3-x}O_4 with x <= 0.7). Dissolution and renucleation/growth occurred during digestion. For larger particles, the magnetizations were the same as for the bulk of the phases present, while the coercivities were more system dependent. We have found that nanoscale particles, on the other hand, showed profound size effects. The saturation magnetization of

  10. Inverse Dipolar Magnetic Anomaly Over the Volcanic Cone Linked to Reverse Polarity Magnetizations in Lavas and Tuffs - Implications for the Conduit System

    NASA Astrophysics Data System (ADS)

    Fucugauchi, J. U.; Perez-Cruz, L. L.; Trigo-Huesca, A.

    2012-12-01

    A combined magnetics and paleomagnetic study of Toluquilla monogenetic volcano and associated lavas and tuffs from Valsequillo basin in Central Mexico provides evidence on a magnetic link between lavas, ash tuffs and the underground volcanic conduit system. Paleomagnetic analyses show that lavas and ash tuffs carry reverse polarity magnetizations, which correlate with the inversely polarized dipolar magnetic anomaly over the volcano. The magnetizations in the lava and tuff show similar southward declinations and upward inclinations, supporting petrological inferences that the tuff was emplaced while still hot and indicating a temporal correlation for lava and tuff emplacement. Conduit geometry is one of the important controlling factors in eruptive dynamics of basaltic volcanoes. However volcanic conduits are often not, or only partly, exposed. Modeling of the dipolar anomaly gives a reverse polarity source magnetization associated with a vertical prismatic body with southward declination and upward inclination, which correlates with the reverse polarity magnetizations in the lava and tuff. The study documents a direct correlation of the paleomagnetic records with the underground magmatic conduit system of the monogenetic volcano. Time scale for cooling of the volcanic plumbing system involves a longer period than the one for the tuff and lava, suggesting that magnetization for the source of dipolar anomaly may represent a long time average as compared to the spot readings in the lava and tuff. The reverse polarity magnetizations in lava and tuff and in the underground source body for the magnetic anomaly are interpreted in terms of eruptive activity of Toluquilla volcano at about 1.3 Ma during the Matuyama reverse polarity C1r.2r chron.

  11. Magnetic properties of frictional volcanic materials

    NASA Astrophysics Data System (ADS)

    Kendrick, Jackie E.; Lavallée, Yan; Biggin, Andrew; Ferk, Annika; Leonhardt, Roman

    2015-04-01

    During dome-building volcanic eruptions, highly viscous magma extends through the upper conduit in a solid-like state. The outer margins of the magma column accommodate the majority of the strain, while the bulk of the magma is able to extrude, largely undeformed, to produce magma spines. Spine extrusion is often characterised by the emission of repetitive seismicity, produced in the upper <1 km by magma failure and slip at the conduit margins. The rheology of the magma controls the depth at which fracture can occur, while the frictional properties of the magma are important in controlling subsequent marginal slip processes. Upon extrusion, spines are coated by a carapace of volcanic fault rocks which provide insights into the deeper conduit processes. Frictional samples from magma spines at Mount St. Helens (USA), Soufriere Hills (Montserrat) and Mount Unzen (Japan) have been examined using structural, thermal and magnetic analyses to reveal a history of comminution, frictional heating, melting and cooling to form volcanic pseudotachylyte. Pseudotachylyte has rarely been noted in volcanic materials, and the recent observation of its syn-eruptive formation in dome-building volcanoes was unprecedented. The uniquely high thermal conditions of volcanic environments means that frictional melt remains at elevated temperatures for longer than usual, causing slow crystallisation, preventing the development of some signature "quench" characteristics. As such, rock-magnetic tests have proven to be some of the most useful tools in distinguishing pseudotachylytes from their andesite/ dacite hosts. In volcanic pseudotachylyte the mass normalised natural remanent magnetisation (NRM) when further normalised with the concentration dependent saturation remanence (Mrs) was found to be higher than the host rock. Remanence carriers are defined as low coercive materials across all samples, and while the remanence of the host rock displays similarities to an anhysteretic remanent

  12. Loess 10Be evidence for an asynchronous Brunhes-Matuyama magnetic polarity reversal

    NASA Astrophysics Data System (ADS)

    Zhou, W.; Beck, W.; Kong, X.; An, Z.; Qiang, X.; Wu, Z.; Xian, F.; Ao, H.

    2015-12-01

    In Chinese loess the Brunhes-Matuyama (B-M) geomagnetic reversal appears to occur about 25 ka prior to the established axial dipole reversal age found in many marine sediments, i.e., in Chinese loess this magnetic reversal boundary is found in glacial loess unit L8 which is thought to be correlated with Marine Isotope Stage 20 (MIS 20), in marine sediment records, however, this boundary is commonly found in interglacial period of MIS 19[1-2], leading to the debate on uncertainties of paleoclimatic correlation between the Chinese loess-paleosol sequences and marine sediments[3-5]. Based on this issue, here we propose to use the cosmogenic 10Be to address this conundrum. 10Be is a long-lived radionuclide produced in the atmosphere by cosmic ray spallation reactions and carried to the ground attached to aerosols. Its atmospheric production rate is inversely proportional to the geomagnetic field intensity [6]. This allows us to reconstruct past geomagnetic field intensity variations using 10Be concentrations recorded in different sedimentary archives. We carried out both the 10Be studies and paleogeomagnetic measurements in Luochuan and Xifeng sections in Chinese Loess Plateau. Both loess profiles show that 10Be production rate was at a maximum-an indication of the dipole field reversal-at ca. 780 ± 3 ka BP., in paleosol unit S7 corresponding to MIS 19, proving that the timing of B-M reversal recorded in Chinese loess is synchronous with that seen in marine records [1]. These results reaffirmed the conventional paleoclimatic correlation of loess-paleosol sequences with marine isotope stages and the standard loess timescale as correct. However, it is ~25 ka younger than the age (depth) of the paleogeomagnetic measurements, which show that the B-M boundary is in L8 in these two Chinese loess-paleosol sequences, demonstrating that loess magnetic overprinting has occurred. 1.Tauxe, L., et al., 1996, EARTH PLANET SC LETT, 140, 133-1462.Zhou, L.P., and Shackleton, 1999

  13. Correlation between magnetic properties and the hardness of powder steels

    SciTech Connect

    Ul`yanov, A.I.; Merzlyakov, E.F.; Faizullin, R.G.

    1994-07-01

    Density and carbon content are studied for their effect on strength (hardness) and magnetic (coercive force, saturation magnetization) properties of powder steels ZhGr1 and ZhGr1D3. It is shown that the hardness of articles made of these steels may be determined indirectly by measuring two magnetic characteristics.

  14. Regular flow reversals in Rayleigh-Bénard convection in a horizontal magnetic field.

    PubMed

    Tasaka, Yuji; Igaki, Kazuto; Yanagisawa, Takatoshi; Vogt, Tobias; Zuerner, Till; Eckert, Sven

    2016-04-01

    Magnetohydrodynamic Rayleigh-Bénard convection was studied experimentally using a liquid metal inside a box with a square horizontal cross section and aspect ratio of five. Systematic flow measurements were performed by means of ultrasonic velocity profiling that can capture time variations of instantaneous velocity profiles. Applying a horizontal magnetic field organizes the convective motion into a flow pattern of quasi-two-dimensional rolls arranged parallel to the magnetic field. The number of rolls has the tendency to decrease with increasing Rayleigh number Ra and to increase with increasing Chandrasekhar number Q. We explored convection regimes in a parameter range, at 2×10^{3}reversals in which five rolls periodically change the direction of their circulation with gradual skew of the roll axes can be considered as the most remarkable one. The regime appears around a range of Ra/Q=10, where irregular flow reversals were observed in Yanagisawa et al. We performed the proper orthogonal decomposition (POD) analysis on the spatiotemporal velocity distribution and detected that the regular flow reversals can be interpreted as a periodic emergence of a four-roll state in a dominant five-roll state. The POD analysis also provides the definition of the effective number of rolls as a more objective approach. PMID:27176392

  15. Regular flow reversals in Rayleigh-Bénard convection in a horizontal magnetic field

    NASA Astrophysics Data System (ADS)

    Tasaka, Yuji; Igaki, Kazuto; Yanagisawa, Takatoshi; Vogt, Tobias; Zuerner, Till; Eckert, Sven

    2016-04-01

    Magnetohydrodynamic Rayleigh-Bénard convection was studied experimentally using a liquid metal inside a box with a square horizontal cross section and aspect ratio of five. Systematic flow measurements were performed by means of ultrasonic velocity profiling that can capture time variations of instantaneous velocity profiles. Applying a horizontal magnetic field organizes the convective motion into a flow pattern of quasi-two-dimensional rolls arranged parallel to the magnetic field. The number of rolls has the tendency to decrease with increasing Rayleigh number Ra and to increase with increasing Chandrasekhar number Q . We explored convection regimes in a parameter range, at 2 ×103reversals in which five rolls periodically change the direction of their circulation with gradual skew of the roll axes can be considered as the most remarkable one. The regime appears around a range of Ra /Q =10 , where irregular flow reversals were observed in Yanagisawa et al. We performed the proper orthogonal decomposition (POD) analysis on the spatiotemporal velocity distribution and detected that the regular flow reversals can be interpreted as a periodic emergence of a four-roll state in a dominant five-roll state. The POD analysis also provides the definition of the effective number of rolls as a more objective approach.

  16. Regular flow reversals in Rayleigh-Bénard convection in a horizontal magnetic field.

    PubMed

    Tasaka, Yuji; Igaki, Kazuto; Yanagisawa, Takatoshi; Vogt, Tobias; Zuerner, Till; Eckert, Sven

    2016-04-01

    Magnetohydrodynamic Rayleigh-Bénard convection was studied experimentally using a liquid metal inside a box with a square horizontal cross section and aspect ratio of five. Systematic flow measurements were performed by means of ultrasonic velocity profiling that can capture time variations of instantaneous velocity profiles. Applying a horizontal magnetic field organizes the convective motion into a flow pattern of quasi-two-dimensional rolls arranged parallel to the magnetic field. The number of rolls has the tendency to decrease with increasing Rayleigh number Ra and to increase with increasing Chandrasekhar number Q. We explored convection regimes in a parameter range, at 2×10^{3}reversals in which five rolls periodically change the direction of their circulation with gradual skew of the roll axes can be considered as the most remarkable one. The regime appears around a range of Ra/Q=10, where irregular flow reversals were observed in Yanagisawa et al. We performed the proper orthogonal decomposition (POD) analysis on the spatiotemporal velocity distribution and detected that the regular flow reversals can be interpreted as a periodic emergence of a four-roll state in a dominant five-roll state. The POD analysis also provides the definition of the effective number of rolls as a more objective approach.

  17. Extreme Driving of Reverse Convection During Strongly Northward Interplanetary Magnetic Field

    NASA Astrophysics Data System (ADS)

    Clauer, C. R.; Xu, Z.; Hartinger, M.; Maimaiti, M.; Ruohoniemi, J. M.; Scales, W.; Nicolls, M. J.; Wilder, F. D.

    2015-12-01

    A variety of statistical studies have shown that the ionospheric polar potential produced by solar wind - magnetosphere - ionosphere coupling is linear for weak to moderate solar wind driving, but becomes non-linear during periods of very strong driving. It has been shown that this applies to the two-cell convection potential that develops during southward interplanetary magnetic field (IMF) and also to the reverse convection cells that develop during northward IMF. This has been described as polar potential saturation and it appears to begin when the driving solar wind electric field becomes greater than 3 mV/m. It has also been shown that the summer ionospheric electric field saturates at about the same value (20 mV/m) for both northward or southward IMF. Recent measurements of the high latitude convection on September 12 - 13, 2014 using the Resolute Incoherent Scatter Radar during periods of large northward IMF show ionospheric electric fields varying between 56 mV/m and 156 mV/m within the dayside reverse convection cells. There is no indication of saturation during these periods of very strong driving. A second set of observations during June 22-24, 2015 of a CME interaction with the Earth's magnetosphere that also produced large northward IMF during the time period when RISR could measure the dayside reverse convection is also investigated. Factors beyond the strength of the driving electric field must play a role in the process that produces polar potential saturation, at least for the case of reverse convection. Results of an investigation of these additional factors will be discussed.

  18. Magnetization reversal in mixed ferrite-chromite perovskites with non magnetic cation on the A-site.

    PubMed

    Billoni, Orlando V; Pomiro, Fernando; Cannas, Sergio A; Martin, Christine; Maignan, Antoine; Carbonio, Raul E

    2016-11-30

    In this work, we have performed Monte Carlo simulations in a classical model for RFe1-x Cr x O3 with R  =  Y and Lu, comparing the numerical simulations with experiments and mean field calculations. In the analyzed compounds, the antisymmetric exchange or Dzyaloshinskii-Moriya (DM) interaction induced a weak ferromagnetism due to a canting of the antiferromagnetically ordered spins. This model is able to reproduce the magnetization reversal (MR) observed experimentally in a field cooling process for intermediate x values and the dependence with x of the critical temperatures. We also analyzed the conditions for the existence of MR in terms of the strength of DM interactions between Fe(3+) and Cr(3+) ions with the x values variations.

  19. Magnetization reversal in mixed ferrite-chromite perovskites with non magnetic cation on the A-site.

    PubMed

    Billoni, Orlando V; Pomiro, Fernando; Cannas, Sergio A; Martin, Christine; Maignan, Antoine; Carbonio, Raul E

    2016-11-30

    In this work, we have performed Monte Carlo simulations in a classical model for RFe1-x Cr x O3 with R  =  Y and Lu, comparing the numerical simulations with experiments and mean field calculations. In the analyzed compounds, the antisymmetric exchange or Dzyaloshinskii-Moriya (DM) interaction induced a weak ferromagnetism due to a canting of the antiferromagnetically ordered spins. This model is able to reproduce the magnetization reversal (MR) observed experimentally in a field cooling process for intermediate x values and the dependence with x of the critical temperatures. We also analyzed the conditions for the existence of MR in terms of the strength of DM interactions between Fe(3+) and Cr(3+) ions with the x values variations. PMID:27661565

  20. Magnetization reversal in mixed ferrite-chromite perovskites with non magnetic cation on the A-site

    NASA Astrophysics Data System (ADS)

    Billoni, Orlando V.; Pomiro, Fernando; Cannas, Sergio A.; Martin, Christine; Maignan, Antoine; Carbonio, Raul E.

    2016-11-01

    In this work, we have performed Monte Carlo simulations in a classical model for RFe1-x Cr x O3 with R  =  Y and Lu, comparing the numerical simulations with experiments and mean field calculations. In the analyzed compounds, the antisymmetric exchange or Dzyaloshinskii-Moriya (DM) interaction induced a weak ferromagnetism due to a canting of the antiferromagnetically ordered spins. This model is able to reproduce the magnetization reversal (MR) observed experimentally in a field cooling process for intermediate x values and the dependence with x of the critical temperatures. We also analyzed the conditions for the existence of MR in terms of the strength of DM interactions between Fe3+ and Cr3+ ions with the x values variations.

  1. Temperature dependence of coercivity and magnetic reversal in SmCo{sub x} thin films

    SciTech Connect

    Andreescu, R.; O'Shea, M.J.

    2005-05-15

    Sm-Co magnets are prepared by sputter deposition with composition SmCo{sub x}, x=5-12.3. A dependence of magnetization, coercivity, and energy product on the thickness for SmCo{sub 5} is found. The thickest samples have the largest values of each of these properties. Increasing the Co content leads to a two-phase system with hard Sm-Co and soft Co phases that are strongly exchange coupled. Large energy products are obtained (up to 17 MG Oe at 400 K and 19 MG Oe at 300 K). The temperature dependence of the coercivity indicates that domain walls are pinned at narrow pin sites.

  2. The magnetic properties of potassium holmium double tungstate

    NASA Astrophysics Data System (ADS)

    Borowiec, M. T.; Dyakonov, V. P.; Khatsko, E. N.; Zayarnyuk, T.; Zubov, E. E.; Szewczyk, A.; Gutowska, M. U.; Rykova, A. I.; Pietosa, J.; Majchrowski, A.; Michalski, E.; Hoffmann, J.-U.; Prokes, K.; Woźniak, K.; Dobrzycki, Ł.; Barański, M.; Domukhovski, V.; Shtyrkhunova, V.; Żmija, J.; Szymczak, H.

    2011-08-01

    The magnetic investigations of potassium holmium double tungstate KHo(WO4)2 have been performed. The results of measurements of magnetic susceptibility and magnetization as a function of temperature (T from 0.3 K up to 100 K) and magnetic field (up to 1.5 T) are presented. A strong anisotropy of magnetic properties was found. The magnetic measurements data were used to calculate the interaction energy. It was shown that the interactions between nearest neighbors Ho3+ ions have antiferromagnetic character.

  3. Injection-Molded Soft Magnets Prepared from Fe-Based Metallic Glass: Mechanical and Magnetic Properties

    NASA Astrophysics Data System (ADS)

    Zhong, Tian; Huang, Ran; Huang, Jia; Ouyang, Wei

    2015-10-01

    The injection-molded metallic glass soft magnet is prepared from the powder of melt-spun ribbon of Fe36Co36B20Si4Nb4 glassy alloy and Nylon 6,6 of wt.% from 5 to 20 via the polymer injection molding technology. The product is characterized by the SEM, mechanical, and magnetic test. The results indicate that this type of materials has comparable mechanical properties and morphological feature with the conventional injection-molded NdFeB magnet and exhibits excellent soft magnetic behaviors. The magnetic properties of the injected magnets are compared with the raw metallic glass, solvent-casted resin bonding magnets, and thermal-treated magnets to confirm that the processing temperature of Nylon injection does not affect the magnetism. The injection technology is a practical processing method to be applied on the metallic glass for potential usage.

  4. Evolution of magnetic properties and exchange interactions in Ru doped YbCrO3.

    PubMed

    Dalal, Biswajit; Sarkar, Babusona; Dev Ashok, Vishal; De, S K

    2016-10-26

    Magnetic properties of YbCr1-x Ru x O3 as a function of temperature and magnetic field have been investigated to explore the intriguing magnetic phenomena in rare-earth orthochromites. A quantitative analysis of x-ray photoelectron spectroscopy confirms the mixed valence state (Yb(3+) and Yb(2+)) of Yb ions for the highest doped sample. Field-cooled magnetization reveals a broad peak around 75 K and then becomes zero at about 20-24 K, due to the antiparallel coupling between Cr(3+) and Yb(3+) moments. An increase of the Ru(4+) ion concentration leads to a slight increase of compensation temperature T comp from 20 to 24 K, but the Néel temperature remains constant. A larger value of the magnetic moment of Yb ions gives rise to negative magnetization at low temperature. An external magnetic field significantly modifies the temperature dependent magnetization. Simulation of temperature dependent magnetization data, below T N, based on the three (two) magnetic sub-lattice model predicts stronger intra-sublattice exchange interaction than that of inter-sublattice. Thermal hysteresis and Arrot plots suggest first order magnetic phase transition. Random substitution of Ru(4+) ion reduces the magnetic relaxation time. Weak ferromagnetic component in canted antiferromagnetic system and negative internal magnetic field cause zero-field-cooled exchange bias effect. Large magnetocrystalline anisotropy associated with Ru creates high coercivity in the Ru doped sample. A maximum value of magnetocaloric effect is found around the antiferromagnetic ordering of Yb(3+) ions. Antiferromagnetic transition at about 120 K and temperature induced magnetization reversal lead to normal and inverse magnetocaloric effects in the same material. PMID:27554537

  5. Evolution of magnetic properties and exchange interactions in Ru doped YbCrO3

    NASA Astrophysics Data System (ADS)

    Dalal, Biswajit; Sarkar, Babusona; Ashok, Vishal Dev; De, S. K.

    2016-10-01

    Magnetic properties of YbCr1-x Ru x O3 as a function of temperature and magnetic field have been investigated to explore the intriguing magnetic phenomena in rare-earth orthochromites. A quantitative analysis of x-ray photoelectron spectroscopy confirms the mixed valence state (Yb3+ and Yb2+) of Yb ions for the highest doped sample. Field-cooled magnetization reveals a broad peak around 75 K and then becomes zero at about 20-24 K, due to the antiparallel coupling between Cr3+ and Yb3+ moments. An increase of the Ru4+ ion concentration leads to a slight increase of compensation temperature T comp from 20 to 24 K, but the Néel temperature remains constant. A larger value of the magnetic moment of Yb ions gives rise to negative magnetization at low temperature. An external magnetic field significantly modifies the temperature dependent magnetization. Simulation of temperature dependent magnetization data, below T N, based on the three (two) magnetic sub-lattice model predicts stronger intra-sublattice exchange interaction than that of inter-sublattice. Thermal hysteresis and Arrot plots suggest first order magnetic phase transition. Random substitution of Ru4+ ion reduces the magnetic relaxation time. Weak ferromagnetic component in canted antiferromagnetic system and negative internal magnetic field cause zero-field-cooled exchange bias effect. Large magnetocrystalline anisotropy associated with Ru creates high coercivity in the Ru doped sample. A maximum value of magnetocaloric effect is found around the antiferromagnetic ordering of Yb3+ ions. Antiferromagnetic transition at about 120 K and temperature induced magnetization reversal lead to normal and inverse magnetocaloric effects in the same material.

  6. Ferrimagnetic Tb-Fe Alloy Thin Films: Composition and Thickness Dependence of Magnetic Properties and All-Optical Switching

    NASA Astrophysics Data System (ADS)

    Hebler, Birgit; Hassdenteufel, Alexander; Reinhardt, Patrick; Karl, Helmut; Albrecht, Manfred

    2016-02-01

    Ferrimagnetic rare earth - transition metal Tb-Fe alloy thin films exhibit a variety of different magnetic properties, which depends strongly on composition and temperature. In this study, first the influence of the film thickness (5 - 85 nm) on the sample magnetic properties was investigated in a wide composition range between 15 at.% and 38 at.% of Tb. From our results, we find that the compensation point, remanent magnetization, and magnetic anisotropy of the Tb-Fe films depend not only on the composition but also on the thickness of the magnetic film up to a critical thickness of about 20-30 nm. Beyond this critical thickness, only slight changes in magnetic properties are observed. This behavior can be attributed to a growth-induced modification of the microstructure of the amorphous films, which affects the short range order. As a result, a more collinear alignment of the distributed magnetic moments of Tb along the out-of-plane direction with film thickness is obtained. This increasing contribution of the Tb sublattice magnetization to the total sample magnetization is equivalent to a sample becoming richer in Tb and can be referred to as an “effective” composition. Furthermore, the possibility of all-optical switching, where the magnetization orientation of Tb-Fe can be reversed solely by circularly polarized laser pulses, was analyzed for a broad range of compositions and film thicknesses and correlated to the underlying magnetic properties.

  7. Morphology control of the magnetization reversal mechanism in Co80Ni20 nanomagnets

    NASA Astrophysics Data System (ADS)

    Mercone, Silvana; Zighem, Fatih; Leridon, Brigitte; Gaul, Audrey; Schoenstein, Frédéric; Jouini, Noureddine

    2015-05-01

    Nanowires with very different size, shape, morphology, and crystal symmetry can give rise to a wide ensemble of magnetic behaviors whose optimization determines their applications in nanomagnets. We present here an experimental work on the shape and morphological dependence of the magnetization reversal mechanism in weakly interacting Co80Ni20 hexagonal-close-packed nanowires. Non-agglomerated nanowires (with length L and diameter d) with a controlled shape going from quasi perfect cylinders to diabolos have been studied inside their polyol solution in order to avoid any oxidation process. The coercive field HC was found to follow a standard behavior and to be optimized for an aspect ratio L/d >15 . Interestingly, an unexpected behavior was observed as function of the head morphology leading to the strange situation where a diabolo shaped nanowire is a better nanomagnet than a cylinder. This paradoxical behavior can be ascribed to the growth-competition between the aspect ratio L/d and the head morphology ratio d/D (D being the head width). Our experimental results clearly show the importance of the independent parameter (t = head thickness) that needs to be considered in addition to the shape aspect ratio ( L/d ) in order to fully describe the nanomagnets magnetic behavior. Micromagnetic simulations well support the experimental results and bring important insights for future optimization of the nanomagnets morphology.

  8. Dynamic phase transition phenomena and magnetization reversal process in uniaxial ferromagnetic nanowires

    NASA Astrophysics Data System (ADS)

    Yüksel, Yusuf

    2015-09-01

    By utilizing the Monte Carlo simulation technique with Metropolis algorithm, we have studied the dynamic phase transition properties such as dynamic hysteresis loops and frequency dispersion of their area in the presence of externally applied oscillating magnetic fields. Particular attention has been paid on the variation of the hysteresis loop area (HLA) curves and their maximal behavior at different temperature regimes. In order to understand the physical mechanism behind the maximum lossy point observed in HLA curves, time series of instantaneous magnetization, as well as micromagnetic domain structures have been provided. Most of the qualitative aspects of the results reported in the present work are shown to be not model-specific type but common phenomenon observed in dynamic magnetic systems.

  9. Influencing the properties of dysprosium single-molecule magnets with phosphorus donor ligands.

    PubMed

    Pugh, Thomas; Tuna, Floriana; Ungur, Liviu; Collison, David; McInnes, Eric J L; Chibotaru, Liviu F; Layfield, Richard A

    2015-01-01

    Single-molecule magnets are a type of coordination compound that can retain magnetic information at low temperatures. Single-molecule magnets based on lanthanides have accounted for many important advances, including systems with very large energy barriers to reversal of the magnetization, and a di-terbium complex that displays magnetic hysteresis up to 14 K and shows strong coercivity. Ligand design is crucial for the development of new single-molecule magnets: organometallic chemistry presents possibilities for using unconventional ligands, particularly those with soft donor groups. Here we report dysprosium single-molecule magnets with neutral and anionic phosphorus donor ligands, and show that their properties change dramatically when varying the ligand from phosphine to phosphide to phosphinidene. A phosphide-ligated, trimetallic dysprosium single-molecule magnet relaxes via the second-excited Kramers' doublet, and, when doped into a diamagnetic matrix at the single-ion level, produces a large energy barrier of 256 cm(-1) and magnetic hysteresis up to 4.4 K. PMID:26130418

  10. Influencing the properties of dysprosium single-molecule magnets with phosphorus donor ligands.

    PubMed

    Pugh, Thomas; Tuna, Floriana; Ungur, Liviu; Collison, David; McInnes, Eric J L; Chibotaru, Liviu F; Layfield, Richard A

    2015-07-01

    Single-molecule magnets are a type of coordination compound that can retain magnetic information at low temperatures. Single-molecule magnets based on lanthanides have accounted for many important advances, including systems with very large energy barriers to reversal of the magnetization, and a di-terbium complex that displays magnetic hysteresis up to 14 K and shows strong coercivity. Ligand design is crucial for the development of new single-molecule magnets: organometallic chemistry presents possibilities for using unconventional ligands, particularly those with soft donor groups. Here we report dysprosium single-molecule magnets with neutral and anionic phosphorus donor ligands, and show that their properties change dramatically when varying the ligand from phosphine to phosphide to phosphinidene. A phosphide-ligated, trimetallic dysprosium single-molecule magnet relaxes via the second-excited Kramers' doublet, and, when doped into a diamagnetic matrix at the single-ion level, produces a large energy barrier of 256 cm(-1) and magnetic hysteresis up to 4.4 K.

  11. Influencing the properties of dysprosium single-molecule magnets with phosphorus donor ligands

    PubMed Central

    Pugh, Thomas; Tuna, Floriana; Ungur, Liviu; Collison, David; McInnes, Eric J.L.; Chibotaru, Liviu F.; Layfield, Richard A.

    2015-01-01

    Single-molecule magnets are a type of coordination compound that can retain magnetic information at low temperatures. Single-molecule magnets based on lanthanides have accounted for many important advances, including systems with very large energy barriers to reversal of the magnetization, and a di-terbium complex that displays magnetic hysteresis up to 14 K and shows strong coercivity. Ligand design is crucial for the development of new single-molecule magnets: organometallic chemistry presents possibilities for using unconventional ligands, particularly those with soft donor groups. Here we report dysprosium single-molecule magnets with neutral and anionic phosphorus donor ligands, and show that their properties change dramatically when varying the ligand from phosphine to phosphide to phosphinidene. A phosphide-ligated, trimetallic dysprosium single-molecule magnet relaxes via the second-excited Kramers' doublet, and, when doped into a diamagnetic matrix at the single-ion level, produces a large energy barrier of 256 cm−1 and magnetic hysteresis up to 4.4 K. PMID:26130418

  12. Resonant vortex-core reversal in magnetic nano-spheres as robust mechanism of efficient energy absorption and emission

    NASA Astrophysics Data System (ADS)

    Kim, Sang-Koog; Yoo, Myoung-Woo; Lee, Jehyun; Lee, Jae-Hyeok; Kim, Min-Kwan

    2016-08-01

    We report on novel vortex-core reversal dynamics in nano-spheres of single-vortex spin configuration as revealed by micromagnetic simulations combined with analytical derivations. When the frequency of an AC magnetic field is tuned to the frequency of the vortex-core precession around the direction of a given static field, oscillatory vortex-core reversals occur, and additionally, the frequency is found to change with both the strength of the applied AC field and the particle size. Such resonant vortex-core reversals in nano-spheres may provide a new and efficient means of energy absorption by, and emission from, magnetic nanoparticles, which system can be effectively implemented in bio-applications such as magnetic hyperthermia.

  13. Resonant vortex-core reversal in magnetic nano-spheres as robust mechanism of efficient energy absorption and emission

    PubMed Central

    Kim, Sang-Koog; Yoo, Myoung-Woo; Lee, Jehyun; Lee, Jae-Hyeok; Kim, Min-Kwan

    2016-01-01

    We report on novel vortex-core reversal dynamics in nano-spheres of single-vortex spin configuration as revealed by micromagnetic simulations combined with analytical derivations. When the frequency of an AC magnetic field is tuned to the frequency of the vortex-core precession around the direction of a given static field, oscillatory vortex-core reversals occur, and additionally, the frequency is found to change with both the strength of the applied AC field and the particle size. Such resonant vortex-core reversals in nano-spheres may provide a new and efficient means of energy absorption by, and emission from, magnetic nanoparticles, which system can be effectively implemented in bio-applications such as magnetic hyperthermia. PMID:27531408

  14. Nano/ultrafine grained austenitic stainless steel through the formation and reversion of deformation-induced martensite: Mechanisms, microstructures, mechanical properties, and TRIP effect

    SciTech Connect

    Shirdel, M.; Mirzadeh, H.; Parsa, M.H.

    2015-05-15

    A comprehensive study was carried out on the strain-induced martensitic transformation, its reversion to austenite, the resultant grain refinement, and the enhancement of strength and strain-hardening ability through the transformation-induced plasticity (TRIP) effect in a commercial austenitic 304L stainless steel with emphasis on the mechanisms and the microstructural evolution. A straightforward magnetic measurement device, which is based on the measurement of the saturation magnetization, for evaluating the amount of strain-induced martensite after cold rolling and reversion annealing in metastable austenitic stainless steels was used, which its results were in good consistency with those of the X-ray diffraction (XRD) method. A new parameter called the effective reduction in thickness was introduced, which corresponds to the reasonable upper bound on the obtainable martensite fraction based on the saturation in the martensitic transformation. By means of thermodynamics calculations, the reversion mechanisms were estimated and subsequently validated by experimental results. The signs of thermal martensitic transformation at cooling stage after reversion at 850 °C were found, which was attributed to the rise in the martensite start temperature due to the carbide precipitation. After the reversion treatment, the average grain sizes were around 500 nm and the nanometric grains of the size of ~ 65 nm were also detected. The intense grain refinement led to the enhanced mechanical properties and observation of the change in the work-hardening capacity and TRIP effect behavior. A practical map as a guidance for grain refining and characterizing the stability against grain growth was proposed, which shows the limitation of the reversion mechanism for refinement of grain size. - Graphical abstract: Display Omitted - Highlights: • Nano/ultrafine grained austenitic stainless steel through martensite treatment • A parameter descriptive of a reasonable upper bound on

  15. Dynamic phase reversal of photo-induced precession of magnetization in ferromagnetic (Ga,Mn)As thin film

    NASA Astrophysics Data System (ADS)

    Li, Hang; Zhang, Xinhui; Liu, Xinyu; Furdyna, Jacek K.

    2015-11-01

    Ultrafast laser-triggered coherent magnetization dynamics in ferromagnetic (Ga,Mn)As films have been investigated by time-resolved magneto-optical spectroscopy. Dynamic phase reversal in the magnetic precession process is observed when the ambient temperature or the external magnetic field is varied. This phenomenon is found to be sensitive to the spontaneous magnetization orientation, and is attributed to the giant magnetic linear dichroism (MLD) effect in (Ga,Mn)As. Our findings suggest that this effect will enable the sensitive measurement of the dynamic phase of in-plane magnetization precession on picosecond time scale in the collective spin excitation in (Ga,Mn)As, thus enabling efficient and ultrafast magneto-optical detection for magnetization dynamics in ferromagnetic semiconductor-based spintronic devices.

  16. Electronic and magnetic properties of nanoribbons

    NASA Astrophysics Data System (ADS)

    Fernando, Gayanath; Zhang, Zhiwei; Kocharian, Armen

    We have performed tight-binding calculations with open boundary conditions on a set of twisted nanoribbons (4x100), monitoring the band structure as a function of the twist angle θ. When this angle is zero, the ribbon is rectangular and when it is 60 degrees, the ribbon is cut from a honeycomb lattice. Depending on the parameters of the tight-binding model and the filling factor, semi-metallic or insulating behavior is observed. We have also studied the electronic structure of such ribbons due to the adsorption of small atoms such as nitrogen, a magnetic field and the Rashba spin-orbit interaction. The role of the adsorbed atoms and the Rashba term with regard to the conducting properties and the symmetry breaking of the ribbons will be discussed in some detail. In addition, the effects of electronic correlations on selected small ribbons will be examined. The authors acknowledge the computing facilities provided by the Center for Functional Nanomaterials, Brookhaven National Laboratory supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886.

  17. Magnetic Properties of Strontium Hexaferrite Nanostructures Measured with Magnetic Force Microscopy

    PubMed Central

    Li, Qiang; Song, Jie; Saura-Múzquiz, Matilde; Besenbacher, Flemming; Christensen, Mogens; Dong, Mingdong

    2016-01-01

    Magnetic property is one of the important properties of nanomaterials. Direct investigation of the magnetic property on the nanoscale is however challenging. Herein we present a quantitative measurement of the magnetic properties including the magnitude and the orientation of the magnetic moment of strontium hexaferrite (SrFe12O19) nanostructures using magnetic force microscopy (MFM) with nanoscale spatial resolution. The measured magnetic moments of the as-synthesized individual SrFe12O19 nanoplatelets are on the order of ~10−16 emu. The MFM measurements further confirm that the magnetic moment of SrFe12O19 nanoplatelets increases with increasing thickness of the nanoplatelet. In addition, the magnetization directions of nanoplatelets can be identified by the contrast of MFM frequency shift. Moreover, MFM frequency imaging clearly reveals the tiny magnetic structures of a compacted SrFe12O19 pellet. This work demonstrates the mesoscopic investigation of the intrinsic magnetic properties of materials has a potential in development of new magnetic nanomaterials in electrical and medical applications. PMID:27174466

  18. Magnetic Properties of Strontium Hexaferrite Nanostructures Measured with Magnetic Force Microscopy.

    PubMed

    Li, Qiang; Song, Jie; Saura-Múzquiz, Matilde; Besenbacher, Flemming; Christensen, Mogens; Dong, Mingdong

    2016-01-01

    Magnetic property is one of the important properties of nanomaterials. Direct investigation of the magnetic property on the nanoscale is however challenging. Herein we present a quantitative measurement of the magnetic properties including the magnitude and the orientation of the magnetic moment of strontium hexaferrite (SrFe12O19) nanostructures using magnetic force microscopy (MFM) with nanoscale spatial resolution. The measured magnetic moments of the as-synthesized individual SrFe12O19 nanoplatelets are on the order of ~10(-16) emu. The MFM measurements further confirm that the magnetic moment of SrFe12O19 nanoplatelets increases with increasing thickness of the nanoplatelet. In addition, the magnetization directions of nanoplatelets can be identified by the contrast of MFM frequency shift. Moreover, MFM frequency imaging clearly reveals the tiny magnetic structures of a compacted SrFe12O19 pellet. This work demonstrates the mesoscopic investigation of the intrinsic magnetic properties of materials has a potential in development of new magnetic nanomaterials in electrical and medical applications. PMID:27174466

  19. Magnetic Properties of Strontium Hexaferrite Nanostructures Measured with Magnetic Force Microscopy

    NASA Astrophysics Data System (ADS)

    Li, Qiang; Song, Jie; Saura-Múzquiz, Matilde; Besenbacher, Flemming; Christensen, Mogens; Dong, Mingdong

    2016-05-01

    Magnetic property is one of the important properties of nanomaterials. Direct investigation of the magnetic property on the nanoscale is however challenging. Herein we present a quantitative measurement of the magnetic properties including the magnitude and the orientation of the magnetic moment of strontium hexaferrite (SrFe12O19) nanostructures using magnetic force microscopy (MFM) with nanoscale spatial resolution. The measured magnetic moments of the as-synthesized individual SrFe12O19 nanoplatelets are on the order of ~10-16 emu. The MFM measurements further confirm that the magnetic moment of SrFe12O19 nanoplatelets increases with increasing thickness of the nanoplatelet. In addition, the magnetization directions of nanoplatelets can be identified by the contrast of MFM frequency shift. Moreover, MFM frequency imaging clearly reveals the tiny magnetic structures of a compacted SrFe12O19 pellet. This work demonstrates the mesoscopic investigation of the intrinsic magnetic properties of materials has a potential in development of new magnetic nanomaterials in electrical and medical applications.

  20. Magnetic Properties of Strontium Hexaferrite Nanostructures Measured with Magnetic Force Microscopy

    NASA Astrophysics Data System (ADS)

    Li, Qiang; Song, Jie; Saura-Múzquiz, Matilde; Besenbacher, Flemming; Christensen, Mogens; Dong, Mingdong

    2016-05-01

    Magnetic property is one of the important properties of nanomaterials. Direct investigation of the magnetic property on the nanoscale is however challenging. Herein we present a quantitative measurement of the magnetic properties including the magnitude and the orientation of the magnetic moment of strontium hexaferrite (SrFe12O19) nanostructures using magnetic force microscopy (MFM) with nanoscale spatial resolution. The measured magnetic moments of the as-synthesized individual SrFe12O19 nanoplatelets are on the order of ~10‑16 emu. The MFM measurements further confirm that the magnetic moment of SrFe12O19 nanoplatelets increases with increasing thickness of the nanoplatelet. In addition, the magnetization directions of nanoplatelets can be identified by the contrast of MFM frequency shift. Moreover, MFM frequency imaging clearly reveals the tiny magnetic structures of a compacted SrFe12O19 pellet. This work demonstrates the mesoscopic investigation of the intrinsic magnetic properties of materials has a potential in development of new magnetic nanomaterials in electrical and medical applications.

  1. Spectral properties of superconductors with ferromagnetically ordered magnetic impurities

    NASA Astrophysics Data System (ADS)

    Persson, Daniel; Shevtsov, Oleksii; Löfwander, Tomas; Fogelström, Mikael

    2015-12-01

    We present a comprehensive theoretical study of thermodynamic properties of superconductors with a dilute concentration of magnetic impurities, with focus on how the properties of the superconducting host change if the magnetic moments of the impurities order ferromagnetically. Scattering off the magnetic impurities leads to the formation of a band of Yu-Shiba-Rusinov states within the superconducting energy gap that drastically influences superconductivity. In the magnetically ordered system, the magnetization displays a sudden drop as a function of the impurity density or magnetic moment amplitude. The drop occurs as the spin-polarized impurity band crosses the Fermi level and is associated with a quantum phase transition first put forward by Sakurai for the single impurity case. Taking into account that the background magnetic field created by the ordered impurity moments enters as a Zeeman shift, we find that the superconducting phase transition changes from second order to first order for high enough impurity concentrations.

  2. Magnetization reversal of a Nd-Cu-infiltrated Nd-Fe-B nanocrystalline magnet observed with small-angle neutron scattering

    SciTech Connect

    Saito, Kotaro Ono, Kanta; Ueno, Tetsuro; Yano, Masao; Shoji, Tetsuya; Sakuma, Noritsugu; Manabe, Akira; Kato, Akira; Harada, Masashi; Keiderling, Uwe

    2015-05-07

    The magnetization reversal process of Nd-Fe-B nanocrystalline magnets infiltrated with Nd-Cu alloy was examined using small-angle neutron scattering (SANS). The magnetic-field dependence of SANS intensity revealed a qualitative difference between Nd-Cu-infiltrated samples and as-deformed samples. Insufficient magnetic isolation along the direction perpendicular to the nominal c-axis is expected from comparable SANS intensities for different ranges of q values along this direction. For small q values near the coercivity field, Nd-Cu-infiltrated samples show a noticeable reduction in SANS intensity along the nominal c-axis, which is parallel to the external magnetic field. This indicates less spatial fluctuation of magnetic moments in Nd-Cu-infiltrated samples, owing to magnetically isolated Nd{sub 2}Fe{sub 14}B grains.

  3. Magnetic bead-based reverse colorimetric immunoassay strategy for sensing biomolecules.

    PubMed

    Gao, Zhuangqiang; Xu, Mingdi; Hou, Li; Chen, Guonan; Tang, Dianping

    2013-07-16

    A novel reverse colorimetric immunoassay (RCIA) strategy was for the first time designed and utilized for sensitive detection of low-abundance protein (prostate-specific antigen, PSA, used in this case) in biological fluids by coupling highly catalytic efficient catalase with magnetic bead-based peroxidase mimics. To construct such a RCIA system, two nanostructures including magnetic beads and gold nanoparticles were first synthesized and functionalized with anti-PSA capture antibody and catalase/anti-PSA detection antibody, respectively. Thereafter, a specific sandwich-type immunoassay format was employed for determination of PSA by using functional gold nanoparticles as enzymatic bioreactors and anti-PSA-conjugated magnetic beads as a colorimetric developer. The carried catalase, followed by the sandwiched immunocomplex, partially consumed the added hydrogen peroxide in the detection solution, which slowed down the catalytic efficiency of magnetic bead-based peroxidase mimics toward TMB/H2O2, thereby weakening the visible color and decreasing the colorimetric density. Different from conventional colorimetric immunoassay, the RCIA method determined the residual hydrogen peroxide in the substrate after consumption. Under the optimal conditions, the developed RCIA exhibited a wide dynamic range of 0.05-20 ng mL(-1) toward PSA with a detection limit of 0.03 ng mL(-1) at the 3Sblank level. Intra- and interassay coefficients of variation were below 6.1% and 9.3%, respectively. Additionally, the methodology was further validated for the analysis of 12 PSA clinical serum specimens, giving results in good accordance with those obtained by the commercially available enzyme-linked immunosorbent assay (ELISA) method.

  4. Unmixing Multi-Component Magnetic Mixtures in Geologic Materials Using First Order Reversal Curve Diagrams

    NASA Astrophysics Data System (ADS)

    Lascu, I.; Harrison, R. J.; Li, Y.; Muraszko, J.; Channell, J. E. T.; Piotrowski, A. M.; Hodell, D. A.; Necula, C.; Panaiotu, C. G.

    2015-12-01

    We have developed a magnetic unmixing method based on principal component analysis (PCA) of first-order reversal curve (FORC) diagrams. PCA provides an objective and robust statistical framework for unmixing, because it represents data variability as a linear combination of a limited number of principal components that are derived purely on the basis of natural variations contained within the dataset. For PCA we have resampled FORC distributions on grids that capture diagnostic signatures of magnetic domain states. Individual FORC diagrams were then recast as linear combinations of end-member (EM) FORC diagrams, located at user-defined positions in PCA space. The EM selection is guided by constraints derived from physical modeling, and is imposed by data scatter. To test our model, we have investigated temporal variations of two EMs in bulk North Atlantic sediment cores collected from the Rockall Trough and the Iberian Continental Margin. Sediments from these sites contain a mixture of magnetosomes and granulometrically distinct detrital magnetite. We have also quantified the spatial variation of three EM components in surficial sediments along the flow path of the North Atlantic Deep Water (NADW). These samples were separated into granulometric fractions, which also assisted in constraining EM definition. The unmixing model reveals systematic variations in EM relative abundance as a function of distance along NADW flow. Finally, we have applied PCA to the combined dataset of Rockall Trough and NADW sediments, which can be recast as a four-EM mixture, providing enhanced discrimination between components. Our method forms the foundation of a general solution to the problem of unmixing multi-component magnetic mixtures, a fundamental task of rock magnetic studies.

  5. Non-resonant fishbone-like modes in tokamak plasmas with reversed magnetic shear

    NASA Astrophysics Data System (ADS)

    Wang, Xian-Qu; Wang, Xiao-Gang

    2016-03-01

    Energetic ion excited non-resonant fishbone-like modes (FLMs) of m / n  >  1 is investigated for reversed magnetic shear configurations. It is found that the mode can be destabilized by trapped fast ions with a similar excitation mechanism as m / n  =  1 fishbones but with a local interchange-like mode structure, which is in agreement with previous experiments (Toi et al 1999 Nucl. Fusion 39 1929). The dispersion relation of the mode is derived for m / n  >  1. The radial mode structure is then studied by numerically solving the eigenvalue equation. Effects of on/off-axis heating, the width of the particle distribution, the beam energy and the energy distribution on the mode are discussed in detail. Nonlinear analysis of the mode is also carried out by a modified predator-prey model.

  6. Magnetic interaction reversal in watermelon nanostructured Cr-doped Fe nanoclusters

    SciTech Connect

    Kaur, Maninder; Qiang, You; Dai, Qilin; Tang, Jinke; Bowden, Mark; Engelhard, Mark; Wu, Yaqiao

    2013-11-11

    Cr-doped core-shell Fe/Fe-oxide nanoclusters (NCs) were synthesized at varied atomic percentages of Cr from 0 at. % to 8 at. %. The low concentrations of Cr (<10 at. %) were selected in order to inhibit the complete conversion of the Fe-oxide shell to Cr{sub 2}O{sub 3} and the Fe core to FeCr alloy. The magnetic interaction in Fe/Fe-oxide NCs (∼25 nm) can be controlled by antiferromagnetic Cr-dopant. We report the origin of σ-FeCr phase at very low Cr concentration (2 at. %) unlike in previous studies, and the interaction reversal from dipolar to exchange interaction in watermelon-like Cr-doped core-shell NCs.

  7. Cardiac Magnetic Resonance Imaging Might Complement Two-Dimensional Echocardiography in the Detection of a Reversible Nonischemic Cardiomyopathy

    PubMed Central

    Madanieh, Raef; Mathew, Shawn; Shah, Pratik; Vatti, Satya K.; Madanieh, Abed; Kosmas, Constantine E.; Vittorio, Timothy J.

    2015-01-01

    We report a case of reversible nonischemic dilated cardiomyopathy in a male in his 60s who presented with an acute heart failure syndrome. Both conventional two-dimensional echocardiography and cardiac magnetic resonance imaging (cMRI) demonstrated severe left ventricular systolic dysfunction; however, both modalities were devoid of significant valvular heart disease as well as the presence of fibrosis, infiltration, inflammation, and scar. After six months of aggressive neurohumoral modulation, there was complete reverse remodeling and normalization of left ventricular function, which highlights the role of cMRI as an adjunct to two-dimensional echocardiography in the detection of a potentially reversible nonischemic cardiomyopathy. PMID:26740746

  8. Magnetization Reversal by Out-of-plane Voltage in BiFeO3-based Multiferroic Heterostructures

    PubMed Central

    Wang, J. J.; Hu, J.M.; Peng, Ren-Ci; Gao, Y.; Shen, Y.; Chen, L. Q.; Nan, C. W.

    2015-01-01

    Voltage controlled 180° magnetization reversal has been achieved in BiFeO3-based multiferroic heterostructures, which is promising for the future development of low-power spintronic devices. However, all existing reports involve the use of an in-plane voltage that is unfavorable for practical device applications. Here, we investigate, using phase-field simulations, the out-of-plane (i.e., perpendicular to heterostructures) voltage controlled magnetism in heterostructures consisting of CoFe nanodots and (110) BiFeO3 thin film or island. It is predicted that the in-plane component of the canted magnetic moment at the CoFe/BiFeO3 interface can be reversed repeatedly by applying a perpendicular voltage across the bottom (110) BiFeO3 thin film, which further leads to an in-plane magnetization reversal in the overlaying CoFe nanodot. The non-volatility of such perpendicular voltage controlled magnetization reversal can be achieved by etching the continuous BiFeO3 film into isolated nanoislands with the same in-plane sizes as the CoFe nanodot. The findings would provide general guidelines for future experimental and engineering efforts on developing the electric-field controlled spintronic devices with BiFeO3-based multiferroic heterostructures. PMID:25995062

  9. Correlation of magnetic properties with deformation in electrical steels

    NASA Astrophysics Data System (ADS)

    Papadopoulou, S.

    2016-03-01

    This paper investigates the utilization of magnetic Barkhausen Noise (MBN) and hysteresis loops methods for the non-destructive characterization of deformed electrical steel samples. For this reason electrical steel samples were subjected to uniaxial tensile tests on elastic and plastic region of deformations. Both the MBN and hysteresis loops were measured. The results shown a strong degradation of the magnetic properties on plastically strains. This was attributed to the irreversible movement of the magnetic domain walls, due to the presence of high dislocation density. The resulting magnetic properties were further evaluated by examining the microstructure of the deformed samples by using scanning electron microscopy.

  10. The Aharanov-Bohm effect, magnetic monopoles and reversal in spin-ice lattices.

    PubMed

    Pollard, Shawn D; Zhu, Yimei

    2013-06-01

    The proof of the Aharonov-Bohm (AB) effect has been one of the most important experiments of the last century and used as essential evidence for the theory of gauge fields. In this article, we look at its fundamental relation to the Dirac monopole and string. Despite the Dirac string being invisible to the AB effect, it can be used to study emergent quasiparticles in condensed matter settings that behave similar to the fundamental monopoles and strings between them. We utilize phase-imaging method based on the AB effect to study the ordering in a one-model system - that of frustrated spin ice - to understand the ordering processes that occur during a magnetic field reversal cycle. The reversal is linked to the propagation of monopole defects linked by flux channels, reminiscent of Dirac strings. Monopole interactions govern the defect densities within the lattice. Furthermore, we exploit these interactions to propose a new ordering method in which high degrees of ground-state ordering can be achieved in a frustrated system.

  11. The Aharanov-Bohm effect, magnetic monopoles and reversal in spin-ice lattices.

    PubMed

    Pollard, Shawn D; Zhu, Yimei

    2013-06-01

    The proof of the Aharonov-Bohm (AB) effect has been one of the most important experiments of the last century and used as essential evidence for the theory of gauge fields. In this article, we look at its fundamental relation to the Dirac monopole and string. Despite the Dirac string being invisible to the AB effect, it can be used to study emergent quasiparticles in condensed matter settings that behave similar to the fundamental monopoles and strings between them. We utilize phase-imaging method based on the AB effect to study the ordering in a one-model system - that of frustrated spin ice - to understand the ordering processes that occur during a magnetic field reversal cycle. The reversal is linked to the propagation of monopole defects linked by flux channels, reminiscent of Dirac strings. Monopole interactions govern the defect densities within the lattice. Furthermore, we exploit these interactions to propose a new ordering method in which high degrees of ground-state ordering can be achieved in a frustrated system. PMID:23549453

  12. Magnetic and magnetothermal properties and the magnetic phase diagram of high purity single crystalline terbium along the easy magnetization direction

    SciTech Connect

    Zverev, V. I.; Tishin, A. M.; Chernyshov, A. S.; Mudryk, Ya; Gschneidner Jr., Karl A.; Pecharsky, Vitalij K.

    2014-01-21

    The magnetic and magnetothermal properties of a high purity terbium single crystal have been re-investigated from 1.5 to 350 K in magnetic fields ranging from 0 to 75 kOe using magnetization, ac magnetic susceptibility and heat capacity measurements. The magnetic phase diagram has been refined by establishing a region of the fan-like phase broader than reported in the past, by locating a tricritical point at 226 K, and by a more accurate definition of the critical fields and temperatures associated with the magnetic phases observed in Tb.

  13. Magnetic and magnetothermal properties and the magnetic phase diagram of high purity single crystalline terbium along the easy magnetization direction.

    PubMed

    Zverev, V I; Tishin, A M; Chernyshov, A S; Mudryk, Ya; Gschneidner, K A; Pecharsky, V K

    2014-02-12

    The magnetic and magnetothermal properties of a high purity terbium single crystal have been re-investigated from 1.5 to 350 K in magnetic fields ranging from 0 to 75 kOe using magnetization, ac magnetic susceptibility and heat capacity measurements. The magnetic phase diagram has been refined by establishing a region of the fan-like phase broader than reported in the past, by locating a tricritical point at 226 K, and by a more accurate definition of the critical fields and temperatures associated with the magnetic phases observed in Tb. PMID:24451321

  14. Magnetic and magnetothermal properties and the magnetic phase diagram of high purity single crystalline terbium along the easy magnetization direction.

    PubMed

    Zverev, V I; Tishin, A M; Chernyshov, A S; Mudryk, Ya; Gschneidner, K A; Pecharsky, V K

    2014-02-12

    The magnetic and magnetothermal properties of a high purity terbium single crystal have been re-investigated from 1.5 to 350 K in magnetic fields ranging from 0 to 75 kOe using magnetization, ac magnetic susceptibility and heat capacity measurements. The magnetic phase diagram has been refined by establishing a region of the fan-like phase broader than reported in the past, by locating a tricritical point at 226 K, and by a more accurate definition of the critical fields and temperatures associated with the magnetic phases observed in Tb.

  15. Enhancement in magnetic properties of magnesium substituted bismuth ferrite nanoparticles

    SciTech Connect

    Xu, Jianlong; Xie, Dan E-mail: RenTL@mail.tsinghua.edu.cn; Teng, Changjiu; Zhang, Xiaowen; Zhang, Cheng; Sun, Yilin; Ren, Tian-Ling E-mail: RenTL@mail.tsinghua.edu.cn; Zeng, Min; Gao, Xingsen; Zhao, Yonggang

    2015-06-14

    We report a potential way to effectively improve the magnetic properties of BiFeO{sub 3} (BFO) nanoparticles through Mg{sup 2+} ion substitution at the Fe-sites of BFO lattice. The high purity and structural changes induced by Mg doping are confirmed by X-ray powder diffractometer and Raman spectra. Enhanced magnetic properties are observed in Mg substituted samples, which simultaneously exhibit ferromagnetic and superparamagnetic properties at room temperature. A physical model is proposed to support the observed ferromagnetism of Mg doped samples, and the superparamagnetic properties are revealed by the temperature dependent magnetization measurements. The improved magnetic properties and soft nature obtained by Mg doping in BFO nanoparticles demonstrate the possibility of BFO nanoparticles to practical applications.

  16. Magnetoresistive properties of nanostructured magnetic metals, manganites, and magnetic semiconductors

    NASA Astrophysics Data System (ADS)

    Solin, N. I.; Romashev, L. N.; Naumov, S. V.; Saranin, A. A.; Zotov, A. V.; Olyanich, D. A.; Kotlyar, V. G.; Utas, O. A.

    2016-02-01

    We consider methods for controlling magnetoresistive parameters of magnetic metal superlattices, manganites, and magnetic semiconductors. By reducing the thickness of ferromagnetic layers in superlattices (e.g., Fe layers in Fe/Cr superlattices), it is possible to form superparamagnetic clustered-layered nanostructures with a magnetoresistance weakly depending on the direction of the external magnetic field, which is very important for applications of such type of materials. Producing Mn vacancies and additionally annealing lanthanum manganites in the oxygen atmosphere, it is possible to increase their magnetoresistance by more than four orders of magnitude. By changing the thickness of p- n junction in the structure of ferromagnetic semiconductors, their magnetoresistance can be increased by 2-3 orders of magnitude.

  17. Radial current density effects on rotating magnetic field current drive in field-reversed configurations

    SciTech Connect

    Clemente, R. A.; Gilli, M.; Farengo, R.

    2008-10-15

    Steady state solutions, suitable for field-reversed configurations (FRCs) sustained by rotating magnetic fields (RMFs) are obtained by properly including three-dimensional effects, in the limit of large FRC elongation, and the radial component of Ohm's law. The steady electrostatic potential, necessary to satisfy Ohm's law, is considered to be a surface function. The problem is analyzed at the midplane of the configuration and it is reduced to the solution of two coupled nonlinear differential equations for the real and imaginary parts of the phasor associated to the longitudinal component of the vector potential. Additional constraints are obtained by requesting that the steady radial current density and poloidal magnetic flux vanish at the plasma boundary which is set at the time-averaged separatrix. The results are presented in terms of the degree of synchronism of the electrons with the RMF and compared with those obtained when radial current effects are neglected. Three important differences are observed when compared with the case without radial current density. First, at low penetration of the RMF into the plasma there is a significant increase in the driven azimuthal current. Second, the RMF amplitude necessary to access the high synchronism regime, starting from low synchronism, is larger and the difference appears to increase as the separatrix to classical skin depth ratio increases. Third, the minimum RMF amplitude necessary to sustain almost full synchronism is reduced.

  18. Distance dependence of magnetic field effect inside confined environment of reverse micelles

    NASA Astrophysics Data System (ADS)

    Sarangi, Manas Kumar; Basu, Samita

    2013-06-01

    In this article, we emphasize on the distance dependence of the magnetic field effect (MFE) on the donoracceptor (D-A) pair inside the confined environment of AOT/H2O/n-heptane reverse micellar (RMs) system. For this study N, N-dimethyl aniline (DMA) is used as an electron donor while the protonated form of Acr is treated as an electron acceptor. We report of the occurrence of an associated excited state proton transfer with the photoinduced electron transfer between Acr and DMA forming corresponding radical pair (RP) and radical ion pairs (RIP). The fate of these reaction products has been tested in the presence of an external magnetic field (˜0.08T) by varying the size of the RMs. The MFE between Acr and DMA has been compared to the results with the earlier reported interactions between Acr and TEA (Chemical Physics Letters, 2011, 506, 205-210). We accentuate the importance of the localization of the D and A inside the RMs, and the intervening distance between the pair to be the critical component for observing substantial MFE.

  19. Simulation Studies of Field-Reversed Configurations with Rotating Magnetic Field Current Drive

    NASA Astrophysics Data System (ADS)

    Belova, E. V.; Davidson, R. C.

    2008-11-01

    Results of 3D kinetic simulations of rotating magnetic field (RMF) current drive in field-reversed configuration (FRC) are presented. Self-consistent hybrid simulations have been performed using the HYM code for even- and odd-parity RMF and different FRC parameters and RMF frequencies. Simulations show that the RMF pushes the plasma radially inward, resulting in a reduced plasma density outside separatrix. Lower plasma density and larger RMF amplitudes result in faster RMF field penetration, in agreement with previous two-fluid studies. Generation of axisymmetric toroidal magnetic field during the RMF current drive has been observed. Numerical study of the effects of the applied RMF field on particle confinement shows that the rate of particle losses increases for RMF frequency close to the ion cyclotron frequency. It is also shown that high-frequency even-parity RMF reduces ion losses when it is fully penetrated. It is also found that fully-penetrated, odd-parity RMF forces particles away from the midplane toward the FRC ends. The observed changes in particle confinement are related to ponderomotive forces. Partially penetrated RMF results in mostly radial ponderomotive forces which improve particle confinement in both cases.

  20. Rotating magnetic field current drive of high-temperature field reversed configurations with high ζ scaling

    NASA Astrophysics Data System (ADS)

    Guo, H. Y.; Hoffman, A. L.; Milroy, R. D.

    2007-11-01

    Greatly reduced recycling and impurity ingestion in the Translation, Confinement, and Sustainment—Upgrade (TCSU) device has allowed much higher plasma temperatures to be achieved in the field reversed configurations (FRC) under rotating magnetic field (RMF) formation and sustainment. The hotter plasmas have higher magnetic fields and much higher diamagnetic electron rotation rates so that the important ratio of average electron rotation frequency to RMF frequency, called ζ, approaches unity, for the first time, in TCSU. A large fraction of the RMF power is absorbed by an as yet unexplained (anomalous) mechanism directly proportional to the square of the RMF magnitude. It becomes of relatively lesser significance as the FRC current increases, and simple resistive heating begins to dominate, but the anomalous absorption is useful for initial plasma heating. Measurements of total absorbed power, and comparisons of applied RMF torque to torque on the electrons due to electron-ion friction under high-ζ operation, over a range of temperatures and fields, have allowed the separation of the classical Ohmic and anomalous heating to be inferred, and cross-field plasma resistivities to be calculated.

  1. The Star Thrust Experiment, rotating magnetic field current drive in the field reversed configuration

    NASA Astrophysics Data System (ADS)

    Miller, Kenneth Elric

    2001-11-01

    The Star Thrust Experiment (STX) has formed and sustained the Field Reversed Configuration (FRC) with a Rotating Magnetic Field (RMF) operated at a strength of 25 G and a frequency of 350 kHz. The RMF was generated with two IGBT switched solid state power supplies capable of delivering 2 MW each. Plasmas were typically 2 m long by 0.2m in radius and consisted of fully ionized deuterium at temperatures of 60 eV and peak densities of 5 × 1018m- 3. The primary diagnostic was an extremely small 24 channel berylia jacketed internal magnetic probe that was used to make measurements as a function of time, radius, and axial position. These measurements when combined with the FRC's unique geometry and equilibrium relationships determined many other important plasma parameters. Axial confining fields of 100 G maintained a true vacuum boundary around the plasma and allowed for the study of FRC RMF equilibrium interactions. Key findings are that the RMF maintained a near zero separatrix pressure, penetrated only partially, and drove strong radial and axial flows. Issues discussed include the importance of the RMF driving an axial current distribution consistent with that of the FRC, possible benefits of varying the average beta condition, and potential RMF antenna length limits set by the tendency of driven axial flows to screen the RMF from the plasma.

  2. Magnetic properties and thermal stability of MnBi/NdFeB hybrid bonded magnets

    SciTech Connect

    Cao, S.; Yue, M.; Yang, Y. X.; Zhang, D. T.; Liu, W. Q.; Zhang, J. X.; Guo, Z. H.; Li, W.

    2011-04-01

    Magnetic properties and thermal stability were investigated for the MnBi/NdFeB (MnBi = 0, 20, 40, 60, 80, and 100 wt.%) bonded hybrid magnets prepared by spark plasma sintering (SPS) technique. Effect of MnBi content on the magnetic properties of the hybrid magnets was studied. With increasing MnBi content, the coercivity of the MnBi/NdFeB hybrid magnets increases rapidly, while the remanence and maximum energy product drops simultaneously. Thermal stability measurement on MnBi magnet, NdFeB magnet, and the hybrid magnet with 20 wt.% MnBi indicates that both the NdFeB magnet and the MnBi/NdFeB hybrid magnet have a negative temperature coefficient of coercivity, while the MnBi magnet has a positive one. The (BH){sub max} of the MnBi/NdFeB magnet (MnBi = 20 wt.%) is 5.71 MGOe at 423 K, which is much higher than 3.67 MGOe of the NdFeB magnet, indicating a remarkable improvement of thermal stability.

  3. Structure and magnetic properties of tetragonal Heusler D022-Mn3Ge compound epitaxial films with high perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Sugihara, A.; Suzuki, K.; Mizukami, S.; Miyazaki, T.

    2015-04-01

    We investigated the structure and magnetic properties of epitaxial films of D022-Mn3Ge tetragonal Heusler like compounds in detail. Epitaxial films with a stoichiometric composition were grown on Cr-buffered single crystalline (0 0 1) MgO substrates using ultra-high vacuum sputtering at different growth temperatures. X-ray diffraction showed that D022-ordered films were formed at growth temperatures of ⩾200 °C. Epitaxial growth was indicated by cross-sectional high-resolution transmission electron microscopy. Nanobeam diffraction patterns from the D022-Mn3Ge film grown at 400 °C suggests the absence of planar defects such as stacking faults and twins in the film. Out-of-plane magnetic hysteresis curves with perfect squareness were observed for the films grown at ⩾300 °C. These films also showed abrupt magnetization reversal at a coercivity of about 1 T, which is higher than that of other thin film materials with perpendicular magnetic anisotropy such as CoPt and FePt. A huge domain diameter in the D022-Mn3Ge films was indicated by the initial magnetization curves that were measured by the polar magneto-optical Kerr effect.

  4. EM Properties of Magnetic Minerals at RADAR Frequencies

    NASA Technical Reports Server (NTRS)

    Stillman, D. E.; Olhoeft, G. R.

    2005-01-01

    Previous missions to Mars have revealed that Mars surface is magnetic at DC frequency. Does this highly magnetic surface layer attenuate RADAR energy as it does in certain locations on Earth? It has been suggested that the active magnetic mineral on Mars is titanomaghemite and/or titanomagnetite. When titanium is incorporated into a maghemite or magnetite crystal, the Curie temperature can be significantly reduced. Mars has a wide range of daily temperature fluctuations (303K - 143K), which could allow for daily passes through the Curie temperature. Hence, the global dust layer on Mars could experience widely varying magnetic properties as a function of temperature, more specifically being ferromagnetic at night and paramagnetic during the day. Measurements of EM properties of magnetic minerals were made versus frequency and temperature (300K- 180K). Magnetic minerals and Martian analog samples were gathered from a number of different locations on Earth.

  5. Comparison of Microinstability Properties for Stellarator Magnetic Geometries

    SciTech Connect

    G. Rewoldt; L.-P. Ku; W.M. Tang

    2005-06-16

    The microinstability properties of seven distinct magnetic geometries corresponding to different operating and planned stellarators with differing symmetry properties are compared. Specifically, the kinetic stability properties (linear growth rates and real frequencies) of toroidal microinstabilities (driven by ion temperature gradients and trapped-electron dynamics) are compared, as parameters are varied. The familiar ballooning representation is used to enable efficient treatment of the spatial variations along the equilibrium magnetic field lines. These studies provide useful insights for understanding the differences in the relative strengths of the instabilities caused by the differing localizations of good and bad magnetic curvature and of the presence of trapped particles. The associated differences in growth rates due to magnetic geometry are large for small values of the temperature gradient parameter n identical to d ln T/d ln n, whereas for large values of n, the mode is strongly unstable for all of the different magnetic geometries.

  6. Magnetic unmixing of first-order reversal curve diagrams using principal component analysis

    NASA Astrophysics Data System (ADS)

    Lascu, Ioan; Harrison, Richard J.; Li, Yuting; Muraszko, Joy R.; Channell, James E. T.; Piotrowski, Alexander M.; Hodell, David A.

    2015-09-01

    We describe a quantitative magnetic unmixing method based on principal component analysis (PCA) of first-order reversal curve (FORC) diagrams. For PCA, we resample FORC distributions on grids that capture diagnostic signatures of single-domain (SD), pseudosingle-domain (PSD), and multidomain (MD) magnetite, as well as of minerals such as hematite. Individual FORC diagrams are recast as linear combinations of end-member (EM) FORC diagrams, located at user-defined positions in PCA space. The EM selection is guided by constraints derived from physical modeling and imposed by data scatter. We investigate temporal variations of two EMs in bulk North Atlantic sediment cores collected from the Rockall Trough and the Iberian Continental Margin. Sediments from each site contain a mixture of magnetosomes and granulometrically distinct detrital magnetite. We also quantify the spatial variation of three EM components (a coarse silt-sized MD component, a fine silt-sized PSD component, and a mixed clay-sized component containing both SD magnetite and hematite) in surficial sediments along the flow path of the North Atlantic Deep Water (NADW). These samples were separated into granulometric fractions, which helped constrain EM definition. PCA-based unmixing reveals systematic variations in EM relative abundance as a function of distance along NADW flow. Finally, we apply PCA to the combined data set of Rockall Trough and NADW sediments, which can be recast as a four-EM mixture, providing enhanced discrimination between components. Our method forms the foundation of a general solution to the problem of unmixing multicomponent magnetic mixtures, a fundamental task of rock magnetic studies.

  7. Effect of the stimulus frequency and pulse number of repetitive transcranial magnetic stimulation on the inter-reversal time of perceptual reversal on the right superior parietal lobule

    NASA Astrophysics Data System (ADS)

    Nojima, Kazuhisa; Ge, Sheng; Katayama, Yoshinori; Ueno, Shoogo; Iramina, Keiji

    2010-05-01

    The aim of this study is to investigate the effect of the stimulus frequency and pulses number of repetitive transcranial magnetic stimulation (rTMS) on the inter-reversal time (IRT) of perceptual reversal on the right superior parietal lobule (SPL). The spinning wheel illusion was used as the ambiguous figures stimulation in this study. To investigate the rTMS effect over the right SPL during perceptual reversal, 0.25 Hz 60 pulse, 1 Hz 60 pulse, 0.5 Hz 120 pulse, 1 Hz 120 pulse, and 1 Hz 240 pulse biphasic rTMS at 90% of resting motor threshold was applied over the right SPL and the right posterior temporal lobe (PTL), respectively. As a control, a no TMS was also conducted. It was found that rTMS on 0.25 Hz 60 pulse and 1 Hz 60 pulse applied over the right SPL caused shorter IRT. In contrast, it was found that rTMS on 1 Hz 240-pulse applied over the right SPL caused longer IRT. On the other hand, there is no significant difference between IRTs when the rTMS on 0.5 Hz 120 pulse and 1 Hz 120 pulse were applied over the right SPL. Therefore, the applying of rTMS over the right SPL suggests that the IRT of perceptual reversal is effected by the rTMS conditions such as the stimulus frequency and the number of pulses.

  8. Enhanced magnetic-field-induced optical properties of nanostructured magnetic fluids by doping nematic liquid crystals

    NASA Astrophysics Data System (ADS)

    Wang, Xiang; Pu, Shengli; Ji, Hongzhu; Yu, Guojun

    2012-05-01

    Ferronematic materials composed of 4-cyano-4'-pentylbiphenyl nematic liquid crystal and oil-based Fe3O4 magnetic fluid were prepared using ultrasonic agitation. The birefringence (Δ n) and figure of merit of optical properties ( Q = Δ n/α, where α is the extinction coefficient) of pure magnetic fluids and the as-prepared ferronematic materials were examined and compared. The figure of merit of optical properties weighs the birefringence and extinction of the materials and is more appropriate to evaluate their optical properties. Similar magnetic-field- and magnetic-particle-concentration-dependent properties of birefringence and figure of merit of optical properties were obtained for the pure magnetic fluids and the ferronematic materials. For the ferronematic materials, the values of Q increase with the volume fractions of nematic liquid crystal under certain fixed field strength and are larger than those of their corresponding pure magnetic fluids at high field region. In addition, the enhancement of Q value increases monotonously with the magnetic field and becomes remarkable when the applied magnetic field is beyond 50 mT. The maximum relative enhanced value of Q R exceeds 6.8% in our experiments. The results of this work may conduce to extend the pragmatic applications of nanostructured magnetic fluids in optical field.

  9. Enhanced magnetic-field-induced optical properties of nanostructured magnetic fluids by doping nematic liquid crystals.

    PubMed

    Wang, Xiang; Pu, Shengli; Ji, Hongzhu; Yu, Guojun

    2012-01-01

    Ferronematic materials composed of 4-cyano-4'-pentylbiphenyl nematic liquid crystal and oil-based Fe3O4 magnetic fluid were prepared using ultrasonic agitation. The birefringence (Δn) and figure of merit of optical properties (Q = Δn/α, where α is the extinction coefficient) of pure magnetic fluids and the as-prepared ferronematic materials were examined and compared. The figure of merit of optical properties weighs the birefringence and extinction of the materials and is more appropriate to evaluate their optical properties. Similar magnetic-field- and magnetic-particle-concentration-dependent properties of birefringence and figure of merit of optical properties were obtained for the pure magnetic fluids and the ferronematic materials. For the ferronematic materials, the values of Q increase with the volume fractions of nematic liquid crystal under certain fixed field strength and are larger than those of their corresponding pure magnetic fluids at high field region. In addition, the enhancement of Q value increases monotonously with the magnetic field and becomes remarkable when the applied magnetic field is beyond 50 mT. The maximum relative enhanced value of QR exceeds 6.8% in our experiments. The results of this work may conduce to extend the pragmatic applications of nanostructured magnetic fluids in optical field. PMID:22587542

  10. Enhanced magnetic-field-induced optical properties of nanostructured magnetic fluids by doping nematic liquid crystals.

    PubMed

    Wang, Xiang; Pu, Shengli; Ji, Hongzhu; Yu, Guojun

    2012-01-01

    Ferronematic materials composed of 4-cyano-4'-pentylbiphenyl nematic liquid crystal and oil-based Fe3O4 magnetic fluid were prepared using ultrasonic agitation. The birefringence (Δn) and figure of merit of optical properties (Q = Δn/α, where α is the extinction coefficient) of pure magnetic fluids and the as-prepared ferronematic materials were examined and compared. The figure of merit of optical properties weighs the birefringence and extinction of the materials and is more appropriate to evaluate their optical properties. Similar magnetic-field- and magnetic-particle-concentration-dependent properties of birefringence and figure of merit of optical properties were obtained for the pure magnetic fluids and the ferronematic materials. For the ferronematic materials, the values of Q increase with the volume fractions of nematic liquid crystal under certain fixed field strength and are larger than those of their corresponding pure magnetic fluids at high field region. In addition, the enhancement of Q value increases monotonously with the magnetic field and becomes remarkable when the applied magnetic field is beyond 50 mT. The maximum relative enhanced value of QR exceeds 6.8% in our experiments. The results of this work may conduce to extend the pragmatic applications of nanostructured magnetic fluids in optical field.

  11. Enhanced magnetic-field-induced optical properties of nanostructured magnetic fluids by doping nematic liquid crystals

    PubMed Central

    2012-01-01

    Ferronematic materials composed of 4-cyano-4′-pentylbiphenyl nematic liquid crystal and oil-based Fe3O4 magnetic fluid were prepared using ultrasonic agitation. The birefringence (Δn) and figure of merit of optical properties (Q = Δn/α, where α is the extinction coefficient) of pure magnetic fluids and the as-prepared ferronematic materials were examined and compared. The figure of merit of optical properties weighs the birefringence and extinction of the materials and is more appropriate to evaluate their optical properties. Similar magnetic-field- and magnetic-particle-concentration-dependent properties of birefringence and figure of merit of optical properties were obtained for the pure magnetic fluids and the ferronematic materials. For the ferronematic materials, the values of Q increase with the volume fractions of nematic liquid crystal under certain fixed field strength and are larger than those of their corresponding pure magnetic fluids at high field region. In addition, the enhancement of Q value increases monotonously with the magnetic field and becomes remarkable when the applied magnetic field is beyond 50 mT. The maximum relative enhanced value of QR exceeds 6.8% in our experiments. The results of this work may conduce to extend the pragmatic applications of nanostructured magnetic fluids in optical field. PMID:22587542

  12. THE MAGNETIZATION DEGREE OF THE OUTFLOW POWERING THE HIGHLY POLARIZED REVERSE-SHOCK EMISSION OF GRB 120308A

    SciTech Connect

    Zhang, Shuai; Jin, Zhi-Ping; Wei, Da-Ming E-mail: dmwei@pmo.ac.cn

    2015-01-01

    GRB 120308A, a long duration γ-ray burst (GRB) detected by Swift, was distinguished by a highly polarized early optical afterglow emission that strongly suggests an ordered magnetic field component in the emitting region. In this work, we model the optical and X-ray emission in the reverse and forward shock scenario and show that the strength of the magnetic field in the reverse-shock region is ∼10 times stronger than that in the forward shock region. Consequently, the outflow powering the highly polarized reverse-shock optical emission was mildly magnetized at a degree of σ ∼ a few percent. Considering the plausible magnetic energy dissipation in both the acceleration and prompt emission phases of the GRB outflow, the afterglow data of GRB 120308A provides us with compelling evidence that, at least for some GRBs, a nonignorable fraction of the energy was released in the form of Poynting flux, confirming the finding first made in the reverse-forward shock emission modeling of the optical afterglow of GRB 990123 by Fan et al. in 2002 and Zhang et al. in 2003.

  13. Geomagnetic Polarity Reversal Model of Deeptow Magnetic Survey in the Southwest Subbasin of South China Sea Ridge

    NASA Astrophysics Data System (ADS)

    Qiu, N.; Sun, Z.; Lin, J.; Li, C. F.; Xu, X.

    2014-12-01

    South China Sea basin, which evolved from Cenozoic continental margin rifting and subsequent seafloor spreading, is a classic example of a marginal sea in Western Pacific. Since the early 1980's, several models have been proposed for the formation of this sea basin. The previous studies were based mainly on the distribution of magnetic anomaly lineation obtained from aerial and shipboard measurements. However, large water depth (over 4.5km) and thick sediment cover (up to 1km or more) make the magnetic anoamaly information not so well displayed in aerial and shipboard data. To better understand the evolution of the sea basin, we increased anomaly amplitudes by collecting magnetic data along deep-tow profiles over the magnetic lineations in the South China Sea oceanic area. The one across the southwest subsea basin was analyzed first. The total field magnetic measurements were processed through filtering, resampling, diurnal variation removal, continuation to a level datum, regional field correction, projection to a common azimuth, and deskewing. A magnetic polarity reversal timescale was constructed by matching deep-tow anomalies with a simple, rectangular block magnetization model with the expansion rate for oceanic crust. We analyzed the spreading duration, rate, asymmetry, and reversal events of Southwest subbasin, in reference to the recent GTS2012 geomagnetic polarity representative data and concluded that the Southwest subbasin opened from around 21.767 Ma and stopped around C5C at about 15.974Ma. The full spreading rate varied from 8 to 40 cm/yr. Spreading is usually asymmetric by showing alternate faster spreading rate in one slab than the other in different time periods. From the comparison, several small reversal were revealed in addition to the standard geomagnetic polarity. These findings helped to understand the evolution of the Southwest subbasin of South China Sea and will also help to establish new reversal discrimination.

  14. Reverse Gyrase from the Hyperthermophilic Bacterium Thermotoga maritima: Properties and Gene Structure

    PubMed Central

    de la Tour, Claire Bouthier; Portemer, Christiane; Kaltoum, Habib; Duguet, Michel

    1998-01-01

    The hyperthermophilic bacterium Thermotoga maritima MSB8 possesses a reverse gyrase whose enzymatic properties are very similar to those of archaeal reverse gyrases. It catalyzes the positive supercoiling of the DNA in an Mg2+- and ATP-dependent process. Its optimal temperature of activity is around 90°C, and it is highly thermostable. We have cloned and DNA sequenced the corresponding gene (T. maritima topR). This is the first report describing the analysis of a gene encoding a reverse gyrase in bacteria. The T. maritima topR gene codes for a protein of 1,104 amino acids with a deduced molecular weight of 128,259, a value in agreement with that estimated from the denaturing gel electrophoresis of the purified enzyme. Like its archaeal homologs, the T. maritima reverse gyrase exhibits helicase and topoisomerase domains, and its sequence matches very well the consensus sequence for six reverse gyrases now available. Phylogenetic analysis shows that all reverse gyrases, including the T. maritima enzyme, form a very homogeneous group, distinct from the type I 5′ topoisomerases of the TopA subfamily, for which we have previously isolated a representative gene in T. maritima (topA). The coexistence of these two distinct genes, coding for a reverse gyrase and an ω-like topoisomerase, respectively, together with the recent description of a gyrase in T. maritima (O. Guipaud, E. Marguet, K. M. Noll, C. Bouthier de la Tour, and P. Forterre, Proc. Natl. Acad. Sci. USA 94:10606–10611, 1977) addresses the question of the control of the supercoiling in this organism. PMID:9440516

  15. Reversible Tuning of Individual Carbon Nanotube Mechanical Properties via Defect Engineering.

    PubMed

    Zhang, Bin; Zhao, Longze; Cheng, Yong; Golberg, Dmitri; Wang, Ming-Sheng

    2016-08-10

    The structural defects that inevitably exist in real-world carbon nanotubes (CNTs) are generally considered undesirable because they break the structural perfection and may result in drastically degraded CNT properties. On the other hand, the deliberate defect introduction can provide a possibility to tailor the tube mechanical properties. Herein, we present a fully controllable technique to handle defects by using in situ transmission electron microscopy (TEM). Young's modulus, quality factor of the resonation and tensile strength of CNTs can be controllably, reversibly, and repeatedly tuned. Parallel high-resolution visualizing of structural defects suggests that the property tuning cycles are primarily attributed to the reversible conversion of defects at the atomic scale: the defects are created in the form of vacancies and interstitials under electron irradiation, and they vanish through the recombination via current-induced annealing. For applications, such as reversible frequency-tuned CNT resonators, this defect-engineering technique is demonstrated to be uniquely precise; the frequency may be tuned with 0.1%/min accuracy, improved by 1 order of magnitude compared with the existing approaches. We believe that these results will be highly valuable in a variety of property-tunable CNT-based composites and devices.

  16. Reversible Tuning of Individual Carbon Nanotube Mechanical Properties via Defect Engineering.

    PubMed

    Zhang, Bin; Zhao, Longze; Cheng, Yong; Golberg, Dmitri; Wang, Ming-Sheng

    2016-08-10

    The structural defects that inevitably exist in real-world carbon nanotubes (CNTs) are generally considered undesirable because they break the structural perfection and may result in drastically degraded CNT properties. On the other hand, the deliberate defect introduction can provide a possibility to tailor the tube mechanical properties. Herein, we present a fully controllable technique to handle defects by using in situ transmission electron microscopy (TEM). Young's modulus, quality factor of the resonation and tensile strength of CNTs can be controllably, reversibly, and repeatedly tuned. Parallel high-resolution visualizing of structural defects suggests that the property tuning cycles are primarily attributed to the reversible conversion of defects at the atomic scale: the defects are created in the form of vacancies and interstitials under electron irradiation, and they vanish through the recombination via current-induced annealing. For applications, such as reversible frequency-tuned CNT resonators, this defect-engineering technique is demonstrated to be uniquely precise; the frequency may be tuned with 0.1%/min accuracy, improved by 1 order of magnitude compared with the existing approaches. We believe that these results will be highly valuable in a variety of property-tunable CNT-based composites and devices. PMID:27454869

  17. Exotic Magnetic Properties in {sup 17}C

    SciTech Connect

    Suzuki, Toshio; Otsuka, Takaharu

    2008-12-15

    Magnetic dipole transitions in {sup 17}C are investigated by shell model calculations. The important role of the tensor interaction for magnetic dipole transitions in this exotic neutron-rich nucleus is pointed out. The recently observed anomalous quenching of the magnetic dipole transition in 1/2{sub 1}{sup +} {yields}3/2{sub g.s.}{sup +} is shown to be well explained by using a modified shell model Hamiltonian that takes full account of the tensor force and monopole corrections in the isospin T=1 channel. The predicted quadrupole moment of {sup 17}C is smaller than the value obtained by conventional shell model Hamiltonians.

  18. Synthesis and Magnetic Properties of CoPt Nanoparticles

    NASA Astrophysics Data System (ADS)

    Trung, Truong Thanh; Nhung, Do Thi; Nam, Nguyen Hoang; Luong, Nguyen Hoang

    2016-07-01

    Magnetic nanoparticles CoPt were prepared by the chemical reduction of cobalt (II) chloride and chloroplatinic acid, then the samples were ultrasonicated for 2 h. After annealing at various temperatures from 400°C to 700°C for 1 h, the samples showed hard magnetic properties with coercivity up to 1.15 kOe at room temperature.

  19. Crystal structure, magnetic properties and advances in hexaferrites: A brief review

    NASA Astrophysics Data System (ADS)

    Jotania, Rajshree

    2014-10-01

    Hexaferrites are hard magnetic materials and specifically ferri-magnetic oxides with hexagonal magnetoplumbite type crystallographic structure. Hexagonal ferrites are used as permanent magnets, high-density perpendicular and magneto-optical recording media, and microwave devices like resonance isolators, filters, circulators, phase shifters because of their high magnetic permeability, high electrical resistivity and moderable permittivity. In addition to these; hexagonal ferrites have excellent chemical stability, mechanical hardness and low eddy current loss at high frequencies. The preparation of hexaferrites is a complicated process. Various experimental techniques like standard ceramic techniques, solvent free synthesis route, co precipitation, salt-melt, ion exchange, sol-gel, citrate synthesis, hydrothermal synthesis, spray drying, water-in-oil microemulsion, reverse micelle etc are used to prepare hexaferrite materials. Structural, dielectric and magnetic properties, crystallite size of hexaferrites depend upon nature of substituted ions, method of preparation, sintering temperature and time. The recent interest is nanotechnology, the development of hexaferrite fibres and composites with carbon nano tubes (CNT). Magnetic properties of some doped and un-doped hexaferrites are discussed here. Recent advances in hexaferrites also highlighted in present paper.

  20. Hydrophilic magnetic nanoclusters with thermo-responsive properties and their drug controlled release

    NASA Astrophysics Data System (ADS)

    Meerod, Siraprapa; Rutnakornpituk, Boonjira; Wichai, Uthai; Rutnakornpituk, Metha

    2015-10-01

    Synthesis and drug controlled release properties of thermo-responsive magnetic nanoclusters grafted with poly(N-isopropylacrylamide) (poly(NIPAAm)) and poly(NIPAAm-co-poly(ethylene glycol) methyl ether methacrylate) (PEGMA) copolymers were described. These magnetic nanoclusters were synthesized via an in situ radical polymerization in the presence of acrylamide-grafted magnetic nanoparticles (MNPs). Poly(NIPAAm) provided thermo-responsive properties, while PEGMA played a role in good water dispersibility to the nanoclusters. The ratios of PEGMA to NIPAAm in the (co)polymerization in the presence of the MNPs were fine-tuned such that the nanoclusters with good water dispersibility, good magnetic sensitivity and thermo responsiveness were obtained. The size of the nanoclusters was in the range of 50-100 nm in diameter with about 100-200 particles/cluster. The nanoclusters were well dispersible in water at room temperature and can be suddenly agglomerated when temperature was increased beyond the lower critical solution temperature (LCST) (32 °C). The release behavior of an indomethacin model drug from the nanoclusters was also investigated. These novel magnetic nanoclusters with good dispersibility in water and reversible thermo-responsive properties might be good candidates for the targeting drug controlled release applications.

  1. Structural inhomogeneity and magnetic properties of strontium hexaferrites

    SciTech Connect

    Pashchenko, V.P.; Samoilenko, Z.A.; Vintonyak, V.M.

    1995-07-01

    The clustered inhomogeneity observed in ferromagnetic materials deepens our concepts of the actual structure of solids and opens new possibilities for controlling their properties. These investigations were made for the purpose of establishment of the relationship between clusterization and magnetic properties of SrO-nFe{sub 2}O{sub 3}, where 5.4 < n < 6.2, metal oxide magnetically hard strontium ferrites.

  2. The effects of magnetic nanoparticle properties on magnetic fluid hyperthermia

    NASA Astrophysics Data System (ADS)

    Kappiyoor, Ravi; Liangruksa, Monrudee; Ganguly, Ranjan; Puri, Ishwar K.

    2010-11-01

    Magnetic fluid hyperthermia (MFH) is a noninvasive treatment that destroys cancer cells by heating a ferrofluid-impregnated malignant tissue with an ac magnetic field while causing minimal damage to the surrounding healthy tissue. The strength of the magnetic field must be sufficient to induce hyperthermia but it is also limited by the human ability to safely withstand it. The ferrofluid material used for hyperthermia should be one that is readily produced and is nontoxic while providing sufficient heating. We examine six materials that have been considered as candidates for MFH use. Examining the heating produced by nanoparticles of these materials, barium-ferrite and cobalt-ferrite are unable to produce sufficient MFH heating, that from iron-cobalt occurs at a far too rapid rate to be safe, while fcc iron-platinum, magnetite, and maghemite are all capable of producing stable controlled heating. We simulate the heating of ferrofluid-loaded tumors containing nanoparticles of the latter three materials to determine their effects on tumor tissue. These materials are viable MFH candidates since they can produce significant heating at the tumor center yet maintain the surrounding healthy tissue interface at a relatively safe temperature.

  3. Studying the reversal mode of the magnetization vector versus applied field angle using generalized magneto-optical ellipsometry

    SciTech Connect

    Pufall, M. R.; Berger, A.

    1999-10-26

    The authors used the technique of vector Generalized Magneto-optical Ellipsometry to study the behavior of the magnetization vector of a 50 Co thin film as a function of external field magnitude and direction. With this method, which determines the both the direction and magnitude of the magnetization, averaged over the 1 mm incident laser beam, they were able to determine the relative contributions of magnetization rotation and domain formation to the reversal of M. The Co sample had a uniaxial in-plane anisotropy. The authors found that when the angle between the applied field and the easy axis was greater than {approximately} 40 degrees, the reversal occurred primarily by rotation of the magnetization, accompanied by a small reduction of the magnitude of M. In this angular region, the critical field-the field at which there is a large jump in the angle of M -- as a function of applied field angle followed a coherent rotation model. However, at applied field angles less than 40 degrees to the easy axis, they found a larger reduction in {vert_bar}M{vert_bar} occurring before and during the jump in the magnetization angle. The jump also occurred at fields much lower than those predicted by the coherent rotation model, indicating a reversal mode initiated by domain formation.

  4. Magnetization reversal process in Fe/Si (001) single-crystalline film investigated by planar Hall effect

    NASA Astrophysics Data System (ADS)

    Ye, Jun; He, Wei; Hu, Bo; Tang, Jin; Zhang, Yong-Sheng; Zhang, Xiang-Qun; Chen, Zi-Yu; Cheng, Zhao-Hua

    2015-02-01

    A planar Hall effect (PHE) is introduced to investigate the magnetization reversal process in single-crystalline iron film grown on a Si (001) substrate. Owing to the domain structure of iron film and the characteristics of PHE, the magnetization switches sharply in an angular range of the external field for two steps of 90° domain wall displacement and one step of 180° domain wall displacement near the easy axis, respectively. However, the magnetization reversal process near the hard axis is completed by only one step of 90° domain wall displacement and then rotates coherently. The magnetization reversal process mechanism near the hard axis seems to be a combination of coherent rotation and domain wall displacement. Furthermore, the domain wall pinning energy and uniaxial magnetic anisotropy energy can also be derived from the PHE measurement. Project supported by the National Basic Research Program of China (Grant Nos. 2011CB921801 and 2012CB933102), the National Natural Science Foundation of China (Grant Nos. 11374350, 11034004, 11274361, 11274033, 11474015, and 61227902), and the Research Fund for the Doctoral Program of Higher Education of China (Grant No. 20131102130005).

  5. Magnetization reversal in Ni/FeF2 heterostructures with the coexistence of positive and negative exchange bias

    NASA Astrophysics Data System (ADS)

    Kovylina, Miroslavna; Morales, Rafael; Labarta, Amílcar; Batlle, Xavier

    2012-12-01

    Magnetization reversal mechanisms are studied in Ni/FeF2 heterostructures with the coexistence of positive and negative exchanged bias (PEB/NEB), showing single and double hysteresis loops (DHL) in magnetoresistance measurements. Micromagnetic simulations show that PEB and NEB domains of a minimum critical size must be introduced in order to reproduce the occurrence of DHLs. The simulations reveal that different magnetic configurations and, hence, different magnetization reversal processes take place in a ferromagnet (FM) on top of minority PEB domains that are either greater or smaller than the critical size. In particular, for the case of DHLs, core reversal of a depthwise domain wall is observed over minority PEB domains when the magnetic field is decreased from positive saturation. As the field is further decreased, a complex domain-wall evolution takes place in the FM, including the dependences of the domain-wall width and domain size on the magnetic field and distance from the antiferromagnet (AF). These effects should be taken into account when the domain size is estimated from data measured by depth-dependent techniques since they average the distribution of domain sizes in the FM for different distances from the AF.

  6. Influence Of Nanoparticles Diameter On Structural Properties Of Magnetic Fluid In Magnetic Field

    NASA Astrophysics Data System (ADS)

    Kúdelčík, Jozef; Bury, Peter; Hardoň, Štefan; Kopčanský, Peter; Timko, Milan

    2015-07-01

    The properties of magnetic fluids depend on the nanoparticle diameter, their concentration and the carrier liquid. The structural changes in magnetic fluids with different nanoparticle diameter based on transformer oils TECHNOL and MOGUL under the effect of a magnetic field and temperature were studied by acoustic spectroscopy. At a linear and jump changes of the magnetic field at various temperatures a continuous change was observed of acoustic attenuation caused by aggregation of the magnetic nanoparticles to structures. From the anisotropy of acoustic attenuation and using the Taketomi theory the basic parameters of the structures are calculated and the impact of nanoparticle diameters on the size of structures is confirmed.

  7. Conformational Plasticity of the NNRTI-Binding Pocket in HIV-1 Reverse Transcriptase: A Fluorine Nuclear Magnetic Resonance Study.

    PubMed

    Sharaf, Naima G; Ishima, Rieko; Gronenborn, Angela M

    2016-07-19

    HIV-1 reverse transcriptase (RT) is a major drug target in the treatment of HIV-1 infection. RT inhibitors currently in use include non-nucleoside, allosteric RT inhibitors (NNRTIs), which bind to a hydrophobic pocket, distinct from the enzyme's active site. We investigated RT-NNRTI interactions by solution (19)F nuclear magnetic resonance (NMR), using singly (19)F-labeled RT proteins. Comparison of (19)F chemical shifts of fluorinated RT and drug-resistant variants revealed that the fluorine resonance is a sensitive probe for identifying mutation-induced changes in the enzyme. Our data show that in the unliganded enzyme, the NNRTI-binding pocket is highly plastic and not locked into a single conformation. Upon inhibitor binding, the binding pocket becomes rigidified. In the inhibitor-bound state, the (19)F signal of RT is similar to that of drug-resistant mutant enzymes, distinct from what is observed for the free state. Our results demonstrate the power of (19)F NMR spectroscopy to characterize conformational properties using selectively (19)F-labeled protein. PMID:27163463

  8. Conformational Plasticity of the NNRTI-Binding Pocket in HIV-1 Reverse Transcriptase: A Fluorine Nuclear Magnetic Resonance Study.

    PubMed

    Sharaf, Naima G; Ishima, Rieko; Gronenborn, Angela M

    2016-07-19

    HIV-1 reverse transcriptase (RT) is a major drug target in the treatment of HIV-1 infection. RT inhibitors currently in use include non-nucleoside, allosteric RT inhibitors (NNRTIs), which bind to a hydrophobic pocket, distinct from the enzyme's active site. We investigated RT-NNRTI interactions by solution (19)F nuclear magnetic resonance (NMR), using singly (19)F-labeled RT proteins. Comparison of (19)F chemical shifts of fluorinated RT and drug-resistant variants revealed that the fluorine resonance is a sensitive probe for identifying mutation-induced changes in the enzyme. Our data show that in the unliganded enzyme, the NNRTI-binding pocket is highly plastic and not locked into a single conformation. Upon inhibitor binding, the binding pocket becomes rigidified. In the inhibitor-bound state, the (19)F signal of RT is similar to that of drug-resistant mutant enzymes, distinct from what is observed for the free state. Our results demonstrate the power of (19)F NMR spectroscopy to characterize conformational properties using selectively (19)F-labeled protein.

  9. Origin of the magnetic-field controlled polarization reversal in multiferroic TbMn2 O 5

    NASA Astrophysics Data System (ADS)

    Leo, N.; Meier, D.; Pisarev, R. V.; Park, S.; Cheong, S.-W.; Fiebig, M.

    2011-03-01

    The interplay of multi-dimensional complex magnetic order parameters leads to interesting effects like magnetically induced ferroelectricity. A particular interesting example is TbMn 2 O5 because of the associated magnetic-field controllable electric polarization. By optical second harmonic generation we show that the gigantic magnetoelectric effect originates in three independent ferroelectric contributions. Two of these are manganese-generated. The third contribution is related to the magnetism of the Tb 3+ sublattice and has not been identified so far. It mediates the remarkable magnetic-field induced polarization reversal. This model is verified by experiments on the isostructural YMn 2 O5 where Y3+ ions are nonmagnetic and only two polarization contributions are present and no magnetoelectric coupling is observed. These results underline the importance of the 3 d - 4 f -interaction for the intricate magnetoelectric coupling in the class of isostructural RMn 2 O5 compounds. This work was supported by the DFG through SFB 608.

  10. Magnetic properties of MoS2: Existence of ferromagnetism

    NASA Astrophysics Data System (ADS)

    Tongay, Sefaattin; Varnoosfaderani, Sima S.; Appleton, Bill R.; Wu, Junqiao; Hebard, Arthur F.

    2012-09-01

    We report on the magnetic properties of MoS2 measured from room temperature down to 10 K and magnetic fields up to 5 T. We find that single crystals of MoS2 display ferromagnetism superimposed onto large temperature-dependent diamagnetism and have observed that ferromagnetism persists from 10 K up to room temperature. We attribute the existence of ferromagnetism partly to the presence of zigzag edges in the magnetic ground state at the grain boundaries. Since the magnetic measurements are relatively insensitive to the interlayer coupling, these results are expected to be valid in the single layer limit.

  11. Thermal to electricity conversion using thermal magnetic properties

    DOEpatents

    West, Phillip B [Idaho Falls, ID; Svoboda, John [Idaho Falls, ID

    2010-04-27

    A system for the generation of Electricity from Thermal Energy using the thermal magnetic properties of a Ferromagnetic, Electrically Conductive Material (FECM) in one or more Magnetic Fields. A FECM is exposed to one or more Magnetic Fields. Thermal Energy is applied to a portion of the FECM heating the FECM above its Curie Point. The FECM, now partially paramagnetic, moves under the force of the one or more Magnetic Fields. The movement of the FECM induces an electrical current through the FECM, generating Electricity.

  12. Magnetic Properties of Iron Clusters in Silver

    NASA Astrophysics Data System (ADS)

    Elzain, M.; Al Rawas, A.; Yousif, A.; Gismelseed, A.; Rais, A.; Al-Omari, I.; Bouziane, K.; Widatallah, H.

    2004-12-01

    The discrete variational method is used to study the effect of interactions of iron impurities on the magnetic moments, hyperfine fields and isomer shifts at iron sites in silver. We study small clusters of iron atoms as they grow to form FCC phase that is coherent with the silver lattice. The effects of the lattice relaxation and the ferromagnetic and antiferromagnetic couplings are also considered. When Fe atoms congregate around a central Fe atom in an FCC arrangement under ferromagnetic coupling, the local magnetic moment and the contact charge density at the central atom hardly change as the cluster builds up, whereas the hyperfine field increases asymptotically as the number of Fe nearest neighbors increases. Introduction of antiferromagnetic coupling has minor effect on the local magnetic moments and isomer shifts, however it produces large reduction in the hyperfine field. The lattice relaxation of the surrounding Fe atoms towards a BCC phase around a central Fe atom leads to reduction in the magnetic moment accompanied by increase in the magnetic hyperfine field.

  13. Magnetic properties of Cr 2[Ni 2(CN) 4] 3

    NASA Astrophysics Data System (ADS)

    Juszczyk, S.; Johansson, C.; Hanson, M.; Małecki, G.

    1994-09-01

    We have studied the magnetic properties of Cr 2[Ni 2(CN) 4] 3 in the temperature range 4.2-260 K with the use of fields of up to 12 T. From the magnetization versus temperature curve we have obtained the Curie as well as the Curie-Weiss temperatures, the Curie constant and the effective magnetic moment in the paramagnetic state. From the magnetization curve at T = 10.4 K we have determined the high-field susceptibility. The data suggest that the Cr and Ni cations are magnetic and their sublattices are coupled antiferromagnetically. The properties of the compound are discussed in the framework of the mean field theory.

  14. Reverse polarity magnetized melt rocks from the Chicxulub impact structure, Yucatan Peninsula, Mexico

    NASA Technical Reports Server (NTRS)

    Urrutia-Fucugauchi, Jaime; Marin, Luis E.; Sharpton, Virgil L.; Quezada, Juan Manuel

    1993-01-01

    Further paleomagnetic data for core samples of melt rock recovered in the Petroleos Mexicanos (PEMEX) exploratory wells within the Chicxulub structure, northern Yucatan peninsula, Mexico are reported. A previous report by Sharpton showed that the rocks studied contain high iridium levels and shocked breccia clasts, and an Ar-40/Ar-39 age of 65.2 plus or minus 0.4 Ma. The geomagnetic polarity determined for two samples is reverse (R) and was correlated with chron 29R that includes the K/T boundary. Our present analysis is based on two samples from each of three clasts of the melt rock from PEMEX well Y6-N17 (1295 to 1299 m b.s.l.). This study concentrates on the vectorial nature and stability of the remanence (NRM), the magnetic mineralogy and remanence carriers (i.e., the reliability and origin of the record), and on the implications (correlation with expected paleolatitude and polarity). The relative orientation of the drill core samples with respect to the horizontal is known. Samples were stable under alternating field (AF) and thermal treatments, and after removal of a small component they exhibited single-vectorial behavior. The characteristic remanence inclinations show small dispersion and a mean value (-43 deg) in close agreement with the expected inclination and paleolatitude (derived from the North American apparent polar wander path). Isothermal remenence (IRM) acquisition experiments, Lowrie-Fuller tests, coercivity and unblocking temperature spectra of NRM and saturation IRM, susceptibility and Q-coefficient analyses, and the single-component nature indicate a dominant mineralogy of iron-rich titanomagnetites with single or pseduo-single domain states. The stable characteristic magnetization may be interpreted as a result of shock heating of the rock at the time of formation of the inpact structure and its polarity, age, and paleolatitude are consistent with a time about the K/T boundary.

  15. Passive Superconducting Flux Conservers for Rotating-Magnetic-Field-Driven Field-Reversed Configurations

    SciTech Connect

    Oz, E.; Myers, C. E.; Edwards, M. R.; Berlinger, B.; Brooks, A.; Cohen, S. A.

    2011-01-05

    The Princeton Field-Reversed Configuration (PFRC) experiment employs an odd-parity rotating magnetic field (RMFo) current drive and plasma heating system to form and sustain high-Β plasmas. For radial confinement, an array of coaxial, internal, passive, flux-conserving (FC) rings applies magnetic pressure to the plasma while still allowing radio-frequency RMFo from external coils to reach the plasma. The 3 ms pulse duration of the present experiment is limited by the skin time (τfc) of its room-temperature copper FC rings. To explore plasma phenomena with longer characteristic times, the pulse duration of the next-generation PFRC-2 device will exceed 100 ms, necessitating FC rings with (τfc > 300 ms. In this paper we review the physics of internal, discrete, passive FCs and describe the evolution of the PFRC's FC array. We then detail new experiments that have produced higher performance FC rings that contain embedded high-temperature superconducting (HTS) tapes. Several HTS tape winding configurations have been studied and a wide range of extended skin times, from 0.4 s to over 103 s, has been achieved. The new FC rings must carry up to 3 kA of current to balance the expected PFRC-2 plasma pressure, so the dependence of the HTS-FC critical current on the winding configuration and temperature was also studied. From these experiments, the key HTS-FC design considerations have been identified and HTS-FC rings with the desired performance characteristics have been produced.

  16. Magnetic properties of rare-earth metallofullerenes

    SciTech Connect

    Funasaka, Hideyuki; Sugiyama, Kenji; Yamamoto, Kazunori; Takahashi, Takeshi )

    1995-02-16

    Bulk amounts of La C[sub 82] and Gd C[sub 82] have been isolated in pure form from various hollow fullerenes. Magnetization data for these powder samples, an isolated La C[sub 82] isomer and a Gd C[sub 82] isomer, have been obtained employing a SQUID magnetometer at temperatures ranging from 3 to 300 K. For La C[sub 82] the inverse susceptibility as a function of temperature follows a Curie-Weiss law. The effective magnetic moment per La C[sub 82] is 0.38 [mu][sub B]. For Gd C[sub 32] the magnetization data fall on a universal curve which is fitted to a Brillouin function in correspondence with the Gd[sup 3+] free ion ground state values of J = 3.38 and g = 2. 33 refs., 6 figs.

  17. Magnetic properties on strained manganite thin film

    NASA Astrophysics Data System (ADS)

    Prajapat, C. L.; Singh, M. R.; Gupta, S. K.; Bhattacharya, D.; Basu, S.; Ravikumar, G.

    2014-04-01

    Structural and magnetic studies on La2/3Sr1/3MnO3 (LSMO) epitaxial films grown on STO (100) and MgO (100) substrates by Pulsed Laser Deposition are presented. Due to larger interface strain, the grain size of LSMO on MgO is much smaller than that on STO substrate. However, anisotropy energy produced as a result of in plane tensile strain is much larger in case of the films deposited on MgO in such a way that the blocking (irreversibility) temperature and the coercive fields inferred from temperature and magnetic field dependent magnetization measurements are significantly higher. The importance of this result for the memory applications is highlighted.

  18. Nuclear magnetic resonance properties of lunar samples.

    NASA Technical Reports Server (NTRS)

    Kline, D.; Weeks, R. A.

    1972-01-01

    Nuclear magnetic resonance spectra of Na-23, Al-27, and P-31 in fines samples 10084,60 and 14163,168 and in crystalline rock samples 12021,55 and 14321,166, have been recorded over a range of frequencies up to 20 MHz. A shift in the field at which maximum absorption occurs for all of the spectra relative to the field at which maximum absorption occurs for terrestrial analogues is attributed to a sample-dependent magnetic field at the Na, Al, and P sites opposing the laboratory field. The magnitude of these fields internal to the samples is sample dependent and varies from 5 to 10 G. These fields do not correlate with the iron content of the samples. However, the presence of single-domain particles of iron distributed throughout the plagioclase fraction that contains the principal fraction of Na and Al is inferred from electron magnetic resonance spectra shapes.

  19. Polymer nanocomposites exhibiting magnetically tunable microwave properties

    NASA Astrophysics Data System (ADS)

    Stojak, K.; Pal, S.; Srikanth, H.; Morales, C.; Dewdney, J.; Weller, T.; Wang, J.

    2011-04-01

    Polymer nanocomposites (PNCs) have been synthesized using Rogers polymer and CoFe2O4 nanoparticles (CFO NPs). X-ray diffraction (XRD) confirms the inverse spinel crystal structure of CFO NPs and transmission electron microscopy (TEM) images show the uniform dispersion of nanoparticles (10 nm ± 1) into the polymer matrix. Magnetic measurements indicate superparamagnetic response near room temperature for all PNCs. A blocking temperature TB ~ 298 K was observed and does not vary for different loading fractions of CFO NPs for the PNCs. The saturation magnetization (Ms) was found to be 11 emu g - 1 for 30 wt% CFO, increasing to 32 emu g - 1 for the 80 wt% CFO loaded PNC. A large value of coercivity (Hc = 19 kOe) is also observed at 10 K and is not affected by varying CFO loading. Microwave measurements show significant absorption in the 80 wt% CFO loading PNC and the quality factor shows a strong enhancement with applied magnetic field.

  20. Estimation Model for Magnetic Properties of Stamped Electrical Steel Sheet

    NASA Astrophysics Data System (ADS)

    Kashiwara, Yoshiyuki; Fujimura, Hiroshi; Okamura, Kazuo; Imanishi, Kenji; Yashiki, Hiroyoshi

    Less deterioration in magnetic properties of electrical steel sheets in the process of stamping out iron-core are necessary in order to maintain its performance. First, the influence of plastic strain and stress on magnetic properties was studied by test pieces, in which plastic strain was added uniformly and residual stress was not induced. Because the influence of plastic strain was expressed by equivalent plastic strain, at each equivalent plastic strain state the influence of load stress was investigated. Secondly, elastic limit was determined about 60% of macroscopic yield point (MYP), and it was found to agree with stress limit inducing irreversible deterioration in magnetic properties. Therefore simulation models, where beyond elastic limit plastic deformation begins and magnetic properties are deteriorated steeply, are proposed. Besides considered points in the deformation analysis are strain-rate sensitivity of flow stress, anisotropy under deformation, and influence of stress triaxiality on fracture. Finally, proposed models have been shown to be valid, because magnetic properties of 5mm width rectangular sheets stamped out from non-oriented electrical steel sheet (35A250 JIS grade) can be estimated with good accuracy. It is concluded that the elastic limit must be taken into account in both stamping process simulation and magnetic field calculation.

  1. Reversal magnetization dependence with the Cr and Fe oxidation states in YFe1-xCrxO3 (0≤x≤1) perovskites

    NASA Astrophysics Data System (ADS)

    Fabian, F. A.; Pedra, P. P.; Moura, K. O.; Duque, J. G. S.; Meneses, C. T.

    2016-06-01

    In this work, we have carried out a detailed study of the magnetic and structural properties of YFe1-xCrxO3 (0≤x≤1) samples with orthorhombic structure obtained by co-precipitation method. Analysis of X-ray diffraction data using Rietveld refinement show that all samples present an orthorhombic crystal system with space group Pnma. Besides, we have observed a reduction of unit cell volume with increasing of the Cr concentration. SEM images show the formation of grains of micrometer order. X-ray Absorption near edge spectroscopy (XANES) measurements show a shift of absorption edge which can be indicate there is (i) different oxidation states to Fe and Cr ions and/or (ii) a changing in the point symmetry of Fe and Cr ions to the compounds. The magnetization measurements indicate a continuous decreasing of the magnetic transition temperature as function of chromium doping. The reversal magnetization effect was observed to concentrations around x=0.5. Besides, the deviation of the Curie-Weiss law and a weak ferromagnetic behavior observed at room temperature in the M vs H curves can be attributed to the strong magnetic interactions between the transition metals with different oxidation states.

  2. Extended magnetohydrodynamic simulations of field reversed configuration formation and sustainment with rotating magnetic field current drive

    SciTech Connect

    Milroy, R. D.; Kim, C. C.; Sovinec, C. R.

    2010-06-15

    Three-dimensional simulations of field reversed configuration (FRC) formation and sustainment with rotating magnetic field (RMF) current drive have been performed with the NIMROD code [C. R. Sovinec et al., J. Comput. Phys. 195, 355 (2004)]. The Hall term is a zeroth order effect with strong coupling between Fourier components, and recent enhancements to the NIMROD preconditioner allow much larger time steps than was previously possible. Boundary conditions to capture the effects of a finite length RMF antenna have been added, and simulations of FRC formation from a uniform background plasma have been performed with parameters relevant to the translation, confinement, and sustainment-upgrade experiment at the University of Washington [H. Y. Guo, A. L. Hoffman, and R. D. Milroy, Phys. Plasmas 14, 112502 (2007)]. The effects of both even-parity and odd-parity antennas have been investigated, and there is no evidence of a disruptive instability for either antenna type. It has been found that RMF effects extend considerably beyond the ends of the antenna, and that a large n=0 B{sub t}heta can develop in the open-field line region, producing a back torque opposing the RMF.

  3. Magnetic and Transport Properties of Mn-ion implanted Si

    NASA Astrophysics Data System (ADS)

    Preisler, V.; Ogawa, M.; Han, X.; Wang, K. L.

    2010-01-01

    We investigate the magnetic and transport properties of Mn-ion implanted Si. Both temperature dependent and field dependent measurements of the samples using a SQUID magnometer reveal ferromagnetic properties at room temperature. Magnetotransport measurements show a large positive magnetoresistance up to 4.5 T with no signs of saturation.

  4. Effect of maghemization on the magnetic properties of pseudo-single-domain magnetite particles

    NASA Astrophysics Data System (ADS)

    Almeida, T.; Muxworthy, A. R.; Kasama, T.; Williams, W.; Damsgaard, C.; Frandsen, C.; Pennycook, T. J.; Dunin-Borkowski, R.

    2015-12-01

    magnetic hysteresis measurements, including first-order reversal curve analysis. The coercivity of the grains is shown to increase with reaction temperature up to 180 ºC, but subsequently decreases after heating above 200 ºC; this magnetic behavior is attributed to the growth of a γ-Fe2O3 shell with magnetic properties distinct from the Fe3O4 core.

  5. Giant and reversible room-temperature elastocaloric effect in a single-crystalline Ni-Fe-Ga magnetic shape memory alloy.

    PubMed

    Li, Yang; Zhao, Dewei; Liu, Jian

    2016-01-01

    Good mechanical properties and large adiabatic temperature change render Heusler-type Ni2FeGa-based magnetic shape memory alloys as a promising candidate material for solid-state mechanical cooling application at ambient conditions. Superelastic behavior and associated elastocaloric effect strongly reply on deformation conditions (e.g. applied strain rate and strain level) of stress-induced martensitic transformations. With the aim of developing high-performance elastic cooling materials, in this work, we have carried out a systematic study on a Ni54Fe19Ga27 [420]-oriented single crystal by exploring the interaction between dynamic deformation parameters and thermal response. A giant and reversible adiabatic temperature change of ±7.5 K triggered by a low stress of 30 MPa was achieved. Such a high specific cooling performance thus offers the great advantage for the small scale solid-state mechanical cooling applications. Besides, a significant temporary residual strain effect has been observed at high strain rate, which is unfavorable for reversible elastocaloric effect but can be overcome by reducing stress hysteresis, and/or by elevating initial environmental temperature. The established criterion for the desirable reversible elastocaloric properties goes beyond the present system, and can be applicable for other shape memory alloys used for elastic cooling techniques. PMID:27138030

  6. Giant and reversible room-temperature elastocaloric effect in a single-crystalline Ni-Fe-Ga magnetic shape memory alloy

    PubMed Central

    Li, Yang; Zhao, Dewei; Liu, Jian

    2016-01-01

    Good mechanical properties and large adiabatic temperature change render Heusler-type Ni2FeGa-based magnetic shape memory alloys as a promising candidate material for solid-state mechanical cooling application at ambient conditions. Superelastic behavior and associated elastocaloric effect strongly reply on deformation conditions (e.g. applied strain rate and strain level) of stress-induced martensitic transformations. With the aim of developing high-performance elastic cooling materials, in this work, we have carried out a systematic study on a Ni54Fe19Ga27 [420]-oriented single crystal by exploring the interaction between dynamic deformation parameters and thermal response. A giant and reversible adiabatic temperature change of ±7.5 K triggered by a low stress of 30 MPa was achieved. Such a high specific cooling performance thus offers the great advantage for the small scale solid-state mechanical cooling applications. Besides, a significant temporary residual strain effect has been observed at high strain rate, which is unfavorable for reversible elastocaloric effect but can be overcome by reducing stress hysteresis, and/or by elevating initial environmental temperature. The established criterion for the desirable reversible elastocaloric properties goes beyond the present system, and can be applicable for other shape memory alloys used for elastic cooling techniques. PMID:27138030

  7. Giant and reversible room-temperature elastocaloric effect in a single-crystalline Ni-Fe-Ga magnetic shape memory alloy.

    PubMed

    Li, Yang; Zhao, Dewei; Liu, Jian

    2016-05-03

    Good mechanical properties and large adiabatic temperature change render Heusler-type Ni2FeGa-based magnetic shape memory alloys as a promising candidate material for solid-state mechanical cooling application at ambient conditions. Superelastic behavior and associated elastocaloric effect strongly reply on deformation conditions (e.g. applied strain rate and strain level) of stress-induced martensitic transformations. With the aim of developing high-performance elastic cooling materials, in this work, we have carried out a systematic study on a Ni54Fe19Ga27 [420]-oriented single crystal by exploring the interaction between dynamic deformation parameters and thermal response. A giant and reversible adiabatic temperature change of ±7.5 K triggered by a low stress of 30 MPa was achieved. Such a high specific cooling performance thus offers the great advantage for the small scale solid-state mechanical cooling applications. Besides, a significant temporary residual strain effect has been observed at high strain rate, which is unfavorable for reversible elastocaloric effect but can be overcome by reducing stress hysteresis, and/or by elevating initial environmental temperature. The established criterion for the desirable reversible elastocaloric properties goes beyond the present system, and can be applicable for other shape memory alloys used for elastic cooling techniques.

  8. Giant and reversible room-temperature elastocaloric effect in a single-crystalline Ni-Fe-Ga magnetic shape memory alloy

    NASA Astrophysics Data System (ADS)

    Li, Yang; Zhao, Dewei; Liu, Jian

    2016-05-01

    Good mechanical properties and large adiabatic temperature change render Heusler-type Ni2FeGa-based magnetic shape memory alloys as a promising candidate material for solid-state mechanical cooling application at ambient conditions. Superelastic behavior and associated elastocaloric effect strongly reply on deformation conditions (e.g. applied strain rate and strain level) of stress-induced martensitic transformations. With the aim of developing high-performance elastic cooling materials, in this work, we have carried out a systematic study on a Ni54Fe19Ga27 [420]-oriented single crystal by exploring the interaction between dynamic deformation parameters and thermal response. A giant and reversible adiabatic temperature change of ±7.5 K triggered by a low stress of 30 MPa was achieved. Such a high specific cooling performance thus offers the great advantage for the small scale solid-state mechanical cooling applications. Besides, a significant temporary residual strain effect has been observed at high strain rate, which is unfavorable for reversible elastocaloric effect but can be overcome by reducing stress hysteresis, and/or by elevating initial environmental temperature. The established criterion for the desirable reversible elastocaloric properties goes beyond the present system, and can be applicable for other shape memory alloys used for elastic cooling techniques.

  9. Tuned Magnetic Properties of L10-MnGa/Co(001) Films by Epitaxial Strain

    PubMed Central

    Kim, Dongyoo; Vitos, Levente

    2016-01-01

    We demonstrate that the interface structure has a significant influence on the magnetic state of MnGa/Co films consisting of L10-MnGa on face-centered-cubic Co(001) surface. We reveal an antiferromagnetic to ferromagnetic magnetization reversal as a function of the lateral lattice constant. The magnetization reversal mainly originates from localized states and weak hybridization at interface due to charge redistribution between muffin-tin spheres and interstitial region. The magnetic anisotropy energy of Mn/Co interface system is enhanced with increasing in-plane lattice constant, which is ascribed to the interface interactions and the above magnetization reversal. PMID:26781348

  10. Synthesis and magnetic properties of Ta/NdFeB-based composite microwires

    SciTech Connect

    Szary, P. Périgo, E. A.; Michels, A.; Luciu, I.; Duday, D.; Wirtz, T.; Choquet, P.

    2015-05-07

    Magnetic NdFeB-based microwire composites have been prepared by the direct current magnetron sputtering technique in a specifically designed sputtering chamber for thin-film deposition in wire geometry. As substrate wire material, we have employed steel and Ta. Annealing of the substrate wires during the deposition process was performed by ohmic heating through the application of a direct current. Samples were characterized by means of vibrating sample magnetometry (VSM) and scanning electron microscopy. Best properties have been encountered when using Ta wires as core (substrate) material. The VSM data show a dramatic impact of the current applied during the deposition process on the magnetic properties. For higher current values, i.e., higher annealing temperatures, the wires exhibit a reversal process that is typical for a two-phase system. Moreover, an increase of the coercive field (and remanent magnetization) is observed, which is ascribed to a modification of the magnetic phase present in the sample due to the annealing. We find an indication for the formation of a magnetic easy-axis direction which is azimuthally oriented around the wire axis.

  11. Thermal simulation of magnetization reversals for size-distributed assemblies of core-shell exchange biased nanoparticles

    NASA Astrophysics Data System (ADS)

    Richy, J.; Jay, J.-Ph.; Pogossian, S. P.; Ben Youssef, J.; Sheppard, C. J.; Prinsloo, A. R. E.; Spenato, D.; Dekadjevi, D. T.

    2016-08-01

    A temperature dependent coherent magnetization reversal model is proposed for size-distributed assemblies of ferromagnetic nanoparticles and ferromagnetic-antiferromagnetic (AF) core-shell nanoparticles. The nanoparticles are assumed to be of uniaxial anisotropy and all aligned along their easy axis. The thermal dependence is included by considering thermal fluctuations, implemented via the Néel-Arrhenius theory. Thermal and angular dependence of magnetization reversal loops, coercive field, and exchange-bias field are obtained, showing that ferromagnetic-antiferromagnetic size-distributed exchange-coupled nanoparticles exhibit temperature-dependent asymmetric magnetization reversal. Also, non-monotonic evolutions of exchange-bias and coercive fields with temperature are demonstrated. The angular dependence of coercive field with temperature exhibits a complex behavior, with the presence of an apex, whose position and amplitude are strongly temperature-dependent. The angular dependence of exchange bias with temperature exhibits complex behaviors, which depends on the AF anisotropy and exchange coupling. The resulting angular behavior demonstrates the key role of the size distribution and temperature in the magnetic response of nanoparticles.

  12. Magnetic properties of a classical XY spin dimer in a "planar" magnetic field

    NASA Astrophysics Data System (ADS)

    Ciftja, Orion; Prenga, Dode

    2016-10-01

    Single-molecule magnetism originates from the strong intra-molecular magnetic coupling of a small number of interacting spins. Such spins generally interact very weakly with the neighboring spins in the other molecules of the compound, therefore, inter-molecular spin couplings are negligible. In certain cases the number of magnetically coupled spins is as small as a dimer, a system that can be considered the smallest nanomagnet capable of storing non-trivial magnetic information on the molecular level. Additional interesting patterns arise if the spin motion is confined to a two-dimensional space. In such a scenario, clusters consisting of spins with large-spin values are particularly attractive since their magnetic interactions can be described well in terms of classical Heisenberg XY spins. In this work we calculate exactly the magnetic properties of a nanomagnetic dimer of classical XY spins in a "planar" external magnetic field. The problem is solved by employing a mathematical approach whose idea is the introduction of auxiliary spin variables into the starting expression of the partition function. Results for the total internal energy, total magnetic moment, spin-spin correlation function and zero-field magnetic susceptibility can serve as a basis to understand the magnetic properties of large-spin dimer building blocks.

  13. Final Report on Development of Optimized Field-Reversed Configuration Plasma Formation Techniques for Magnetized Target Fusion

    SciTech Connect

    Lynn, Alan

    2013-11-01

    The University of New Mexico (UNM) proposed a collaboration with Los Alamos National Laboratory (LANL) to develop and test methods for improved formation of field-reversed configuration (FRC) plasmas relevant to magnetized target fusion (MTF) energy research. MTF is an innovative approach for a relatively fast and cheap path to the production of fusion energy that utilizes magnetic confinement to assist in the compression of a hot plasma to thermonuclear conditions by an external driver. LANL is currently pursing demonstration of the MTF concept via compression of an FRC plasma by a metal liner z-pinch in conjunction with the Air Force Research Laboratory in Albuquerque, NM. A key physics issue for the FRC's ultimate success as an MTF target lies in the initial pre-ionization (PI) stage. The PI plasma sets the initial conditions from which the FRC is created. In particular, the PI formation process determines the amount of magnetic flux that can be trapped to form the FRC. A ringing theta pinch ionization (RTPI) technique, such as currently used by the FRX-L device at LANL, has the advantages of high ionization fraction, simplicity (since no additional coils are required), and does not require internal electrodes which can introduce impurities into the plasma. However RTPI has been shown to only trap 50% of the initial bias flux at best and imposes additional engineering constraints on the capacitor banks. The amount of trapped flux plays an important role in the FRC's final equilibrium, transport, and stability properties, and provides increased ohmic heating of the FRC through induced currents as the magnetic field decays. Increasing the trapped flux also provides the route to greatest potential gains in FRC lifetime, which is essential to provide enough time to translate and compress the FRC effectively. In conjunction with LANL we initially planned to develop and test a microwave break- down system to improve the initial PI plasma formation. The UNM team would

  14. A new perspective on self-reversed thermo-remanent magnetization and room-temperature magnetic exchange bias in quenched and annealed ferri-ilmenite solid solutions

    NASA Astrophysics Data System (ADS)

    Robinson, P.; Harrison, R. J.; Fabian, K.; McEnroe, S. A.; Miyajima, N.

    2012-04-01

    In the 1950's, rocks containing ferri-ilmenite solid solutions with compositions X FeTiO3 = 0.53-0.71 were discovered to self-reverse during cooling in a weak field. Such samples played a vexing early role in the history of geomagnetism, because they demonstrably acquire a thermoremanent magnetization (TRM) inverse to the external field, strengthening a common opinion, at that time, that reversed lavas result from a rock-magnetic self-reversal process, while the geomagnetic field polarity itself is constant in time. Early self-reversal models postulated two distinct phases, a subsidiary phase with weak magnetization, and higher Fe content, Curie temperature, and coercivity, referred to as "the x phase", and a dominant phase with a strong magnetization, lower Fe content, Curie T temperature, and coercivity. The "x phase" magnetizes first at higher temperature parallel to the Earth field, and the dominant phase acquires a stronger magnetization at a lower temperature in an orientation opposite to the Earth field, either by direct antiferromagnetic coupling, or as a magnetostatic response to the previously acquired mineral magnetization. Landmark work by Nord and Lawson, on quench and annealing experiments with TEM, showed that, during quench, the solid solution starts to order, but with alternate A and B positioning of Fe and Ti layers. With coarsening, the alternately and chaotically positioned domains merge along antiphase domain boundaries (APBs) that are inherently unstable. With further annealing, boundaries move and are eliminated due to coarsening of some domains and shrinking of others. They showed that quenched, or slightly annealed samples, show self-reversed TRM, but further annealing results in a coarse simple ferrimagnetic phase. They suggested that the "x phase" is represented by the disordered regions along the chemical antiphase boundaries. Harrison visualized a solid solution sample, after quench and coarsening after annealing, which consisted of two

  15. Reversible Structural Swell-Shrink and Recoverable Optical Properties in Hybrid Inorganic-Organic Perovskite.

    PubMed

    Zhang, Yupeng; Wang, Yusheng; Xu, Zai-Quan; Liu, Jingying; Song, Jingchao; Xue, Yunzhou; Wang, Ziyu; Zheng, Jialu; Jiang, Liangcong; Zheng, Changxi; Huang, Fuzhi; Sun, Baoquan; Cheng, Yi-Bing; Bao, Qiaoliang

    2016-07-26

    Ion migration in hybrid organic-inorganic perovskites has been suggested to be an important factor for many unusual behaviors in perovskite-based optoelectronics, such as current-voltage hysteresis, low-frequency giant dielectric response, and the switchable photovoltaic effect. However, the role played by ion migration in the photoelectric conversion process of perovskites is still unclear. In this work, we provide microscale insights into the influence of ion migration on the microstructure, stability, and light-matter interaction in perovskite micro/nanowires by using spatially resolved optical characterization techniques. We observed that ion migration, especially the migration of MA(+) ions, will induce a reversible structural swell-shrink in perovskites and recoverably affect the reflective index, quantum efficiency, light-harvesting, and photoelectric properties. The maximum ion migration quantity in perovskites was as high as approximately 30%, resulting in lattice swell or shrink of approximately 4.4%. Meanwhile, the evidence shows that ion migration in perovskites could gradually accelerate the aging of perovskites because of lattice distortion in the reversible structural swell-shrink process. Knowledge regarding reversible structural swell-shrink and recoverable optical properties may shed light on the development of optoelectronic and converse piezoelectric devices based on perovskites.

  16. Reversible Structural Swell-Shrink and Recoverable Optical Properties in Hybrid Inorganic-Organic Perovskite.

    PubMed

    Zhang, Yupeng; Wang, Yusheng; Xu, Zai-Quan; Liu, Jingying; Song, Jingchao; Xue, Yunzhou; Wang, Ziyu; Zheng, Jialu; Jiang, Liangcong; Zheng, Changxi; Huang, Fuzhi; Sun, Baoquan; Cheng, Yi-Bing; Bao, Qiaoliang

    2016-07-26

    Ion migration in hybrid organic-inorganic perovskites has been suggested to be an important factor for many unusual behaviors in perovskite-based optoelectronics, such as current-voltage hysteresis, low-frequency giant dielectric response, and the switchable photovoltaic effect. However, the role played by ion migration in the photoelectric conversion process of perovskites is still unclear. In this work, we provide microscale insights into the influence of ion migration on the microstructure, stability, and light-matter interaction in perovskite micro/nanowires by using spatially resolved optical characterization techniques. We observed that ion migration, especially the migration of MA(+) ions, will induce a reversible structural swell-shrink in perovskites and recoverably affect the reflective index, quantum efficiency, light-harvesting, and photoelectric properties. The maximum ion migration quantity in perovskites was as high as approximately 30%, resulting in lattice swell or shrink of approximately 4.4%. Meanwhile, the evidence shows that ion migration in perovskites could gradually accelerate the aging of perovskites because of lattice distortion in the reversible structural swell-shrink process. Knowledge regarding reversible structural swell-shrink and recoverable optical properties may shed light on the development of optoelectronic and converse piezoelectric devices based on perovskites. PMID:27386731

  17. Diagnosing the Properties of the Solar Wind using Magnetic Topology

    NASA Astrophysics Data System (ADS)

    Mikic, Z.; Titov, V. S.; Lionello, R.; Downs, C.; Linker, J.; Torok, T.; Riley, P.

    2015-12-01

    Recent work suggests that the topology of the coronal magnetic field plays a key role in the source and properties of the slow solar wind, through the collection of separatrix surfaces and quasi-separatrix layers (QSLs) that define the S-web (Antiochos et al. 2011; Linker et al. 2011; Titov et al. 2011). We have accumulated extensive experience with using the squashing factor Q to analyze the underlying structural skeleton of the coronal magnetic field, to identify magnetic null points, separator field lines, QSLs, and separatrix surfaces, and their relationship with the topology of coronal hole boundaries. This will be extended by implementing slip mapping (Titov et al. 2009) to detect open, closed, and disconnected flux systems that are formed due to magnetic reconnection in a coronal model driven by both the differential rotation and evolution of the photospheric magnetic field. This idea is based on using forward and backward differences in time between the field line mapping expected from ideal MHD motions and the actual mapping to diagnose magnetic reconnection. This technique can identify regions in the photosphere where closed magnetic field lines are about to open (e.g., via interchange reconnection), and conversely, where open field lines are about to close. We will use these concepts to develop tools that relate the changing magnetic topology to the properties of the solar wind, to plan and interpret Solar Probe Plus and Solar Orbiter observations. Research supported by NASA's Living With a Star Program.

  18. Magnetic properties and magnetic hardening mechansim of Pt-Co-B alloys

    NASA Technical Reports Server (NTRS)

    Qiu, Ning; Flanagan, F.; Wittig, James E.

    1994-01-01

    The intrinsic coercivity is found to be maximized in the Pt42Co45B13 ternary alloy which is undercooled and rapidly solidified (quenched using a 70 m/s wheel speed after undercooling), and then annealed (800 C for 2400 min). The same alloy, processed at slower cooling rates and annealed in the same way, has a much larger scale microstructure and a much lower resulting magnetic coercivity. The microstructure which would optimize the coercitvity of this coercivity of this ternary alloy is a completely ordered L1(sub zero) Pt-Co matrix with a submicron magnetic single-domion Co-boride precipitate. The L1(sub zero) phase is highly anistropic magnetically while the Co-boride precipate is somewhat less so. Annealing treatments designed to produced single-domain Co-boride precipitates enhance the coercivity. This suggests that the refined microstructures is responsible for the high coercivities found in the rapidly solidified and annealed alloy. The magnetic domain wall thickness for a Co-boride precipitate is determined from both experimental observation and theoretical calculation in order to evaluate its influence on the coercivity of the alloy. The effects of the pinning of domain walls and the barrier to the nucleation of reverse domains on the coercivity are discussed. Both microstrucutral analysis and theoretical calculation indicate that the high coercivities in the Pt42Co45B13 alloy are due to the difficult nucleation of reverse magnetic domains.

  19. Magnetic Properties of Dipolar Chains in Ferrofluids

    NASA Astrophysics Data System (ADS)

    Avgin, I.; Huber, D. L.

    2014-06-01

    We have investigated the dipole interaction energies per particle and the local dipole field distributions in a frozen-magnetization model of a ferrofluid chain in a saturating magnetic field. A lognormal distribution of particle diameters was assumed. The interaction energies were calculated for one-dimensional arrays of dipoles with moments parallel to the chain. We have computed the energies by various approximations related to the hard sphere particle diameter distribution. A similar approach was followed for the local field distributions. It was found that the energy per particle and mean local field were largely determined by the mean particle diameter, but the distribution of local fields was sensitive to both the mean diameter and the assumptions about spatial correlations between particles of different size. Detailed results are presented for water-soluble Fe3O4/PAA (polyacrylic acid).

  20. The symmetry properties of planetary magnetic fields

    NASA Technical Reports Server (NTRS)

    Raedler, Karl-Heinz; Ness, Norman F.

    1990-01-01

    This paper provides a comparative study of the geometrical structures of the magnetic fields of earth, Jupiter, Saturn, and Uranus, starting from the traditional multipolar representations of these fields. For earth, Jupiter, and Saturn, the centered dipole, quadrupole, and octupole contributions are included, while at Uranus only the dipole and quadrupole contributions are considered. It is found that there are a number of common features of the magnetic fields of earth and Jupiter. Compared to earth and Jupiter, the Saturnian field exhibits not only a high degree of symmetry about the rotation axis but also a high degree of antisymmetry about the equatorial plane. The Uranian field shows strong deviations from both such symmetries. Nevertheless, there remain features common to all four planets.

  1. Basic magnetic properties of bituminous coal

    USGS Publications Warehouse

    Alexander, C.C.; Thorpe, A.N.; Senftle, F.E.

    1979-01-01

    Magnetic susceptibility and other static magnetic parameters have been measured on a number of bituminous coals from various locations in the United States. The paramagnetic Curie constant correlates negatively with carbon concentration on a moisture-free basis. The major contribution to the total paramagnetism comes from the mineral matter rather than from free radicals or broken bonds. Analysis of the data indicates that the specific paramagnetism is generally lower in the mineral matter found in high-ash compared to low-ash coal. A substantial number of the coal specimens tested also had a ferromagnetic susceptibility which appeared to be associated with magnetite. Magnetite and ??-iron spherules, possibly of meteoritic or volcanic origin, were found in several specimens. ?? 1979.

  2. Magnetic and structural properties of fcc/hcp bi-crystalline multilayer Co nanowire arrays prepared by controlled electroplating

    NASA Astrophysics Data System (ADS)

    Pirota, K. R.; Béron, F.; Zanchet, D.; Rocha, T. C. R.; Navas, D.; Torrejón, J.; Vazquez, M.; Knobel, M.

    2011-04-01

    We report on the structural and magnetic properties of crystalline bi-phase Co nanowires, electrodeposited into the pores of anodized alumina membranes, as a function of their length. Co nanowires present two different coexistent crystalline structures (fcc and hcp) that can be controlled by the time of pulsed electrodeposition. The fcc crystalline phase grows at the early stage and is present at the bottom of all the nanowires, strongly influencing their magnetic behavior. Both structural and magnetic characterizations indicate that the length of the fcc phase is constant at around 260-270 nm. X-ray diffraction measurements revealed a strong preferential orientation (texture) in the (1 0-1 0) direction for the hcp phase, which increases the nanowire length as well as crystalline grain size, degree of orientation, and volume fraction of oriented material. The first-order reversal curve (FORC) method was used to infer both qualitatively and quantitatively the complex magnetization reversal of the nanowires. Under the application of a magnetic field parallel to the wires, the magnetization reversal of each region is clearly distinguishable; the fcc phase creates a high coercive contribution without an interaction field, while the hcp phase presents a smaller coercivity and undergoes a strong antiparallel interaction field from neighboring wires.

  3. Nanofluidic Diodes with Dynamic Rectification Properties Stemming from Reversible Electrochemical Conversions in Conducting Polymers.

    PubMed

    Pérez-Mitta, Gonzalo; Marmisollé, Waldemar A; Trautmann, Christina; Toimil-Molares, María Eugenia; Azzaroni, Omar

    2015-12-16

    The use of solid state nanochannels as nanofluidic diodes is currently a topic of large interest in nanotechnology. Particularly, there is a focus in the development of nanochannels with surface functionalities that make them responsive to multiple environmental variables. Here, we present for the first time the construction of electrochemical potential- and pH-responsive nanofluidic diodes using a novel approach based on a controlled electrochemical polymerization of aniline on gold-coated polycarbonate asymmetric nanochannels. The polyaniline-modified nanochannels showed three different levels of reversible ionic rectification corresponding to the degrees of oxidation of the conducting polymer. Our results demonstrate that this strategy enables an accurate and reversible control of the rectification properties due to the well-defined and predictable electrochemical conversion of charged species generated on the pore walls. We envision that these results will create novel avenues to fabricate electrochemically modulated nanofluidic diodes using conducting polymers integrated into single conical nanopores.

  4. Reversible modification of the structural and electronic properties of a boron nitride monolayer by CO intercalation.

    PubMed

    Ng, May Ling; Shavorskiy, Andrey; Rameshan, Christoph; Mikkelsen, Anders; Lundgren, Edvin; Preobrajenski, Alexei; Bluhm, Hendrik

    2015-04-01

    We demonstrate the reversible intercalation of CO between a hexagonal boron nitride (h-BN) monolayer and a Rh(111) substrate above a threshold CO pressure of 0.01 mbar at room temperature. The intercalation of CO results in the flattening of the originally corrugated h-BN nanomesh and an electronic decoupling of the BN layer from the Rh substrate. The intercalated CO molecules assume a coverage and adsorption site distribution comparable to that on the free Rh(111) surface at similar conditions. The pristine h-BN nanomesh is reinstated upon heating to above 625 K. These observations may open up opportunities for a reversible tuning of the electronic and structural properties of monolayer BN films. PMID:25712198

  5. Reversible Control of Nanoparticle Functionalization and Physicochemical Properties by Dynamic Covalent Exchange†

    PubMed Central

    della Sala, Flavio

    2015-01-01

    Abstract Existing methods for the covalent functionalization of nanoparticles rely on kinetically controlled reactions, and largely lack the sophistication of the preeminent oligonucleotide‐based noncovalent strategies. Here we report the application of dynamic covalent chemistry for the reversible modification of nanoparticle (NP) surface functionality, combining the benefits of non‐biomolecular covalent chemistry with the favorable features of equilibrium processes. A homogeneous monolayer of nanoparticle‐bound hydrazones can undergo quantitative dynamic covalent exchange. The pseudomolecular nature of the NP system allows for the in situ characterization of surface‐bound species, and real‐time tracking of the exchange reactions. Furthermore, dynamic covalent exchange offers a simple approach for reversibly switching—and subtly tuning—NP properties such as solvophilicity. PMID:27346895

  6. Reversible Control of Nanoparticle Functionalization and Physicochemical Properties by Dynamic Covalent Exchange**

    PubMed Central

    della Sala, Flavio; Kay, Euan R

    2015-01-01

    Existing methods for the covalent functionalization of nanoparticles rely on kinetically controlled reactions, and largely lack the sophistication of the preeminent oligonucleotide-based noncovalent strategies. Here we report the application of dynamic covalent chemistry for the reversible modification of nanoparticle (NP) surface functionality, combining the benefits of non-biomolecular covalent chemistry with the favorable features of equilibrium processes. A homogeneous monolayer of nanoparticle-bound hydrazones can undergo quantitative dynamic covalent exchange. The pseudomolecular nature of the NP system allows for the in situ characterization of surface-bound species, and real-time tracking of the exchange reactions. Furthermore, dynamic covalent exchange offers a simple approach for reversibly switching—and subtly tuning—NP properties such as solvophilicity. PMID:25973468

  7. Tailoring the magnetic and pharmacokinetic properties of iron oxide magnetic particle imaging tracers

    PubMed Central

    Ferguson, Richard Mathew; Khandhar, Amit P; Arami, Hamed; Hua, Loc; Hovorka, Ondrej; Krishnan, Kannan M.

    2014-01-01

    Magnetic particle imaging (MPI) is an attractive new modality for imaging distributions of iron oxide nanoparticle tracers in vivo. With exceptional contrast, high sensitivity, and good spatial resolution, MPI shows promise for clinical imaging in angiography and oncology. Critically, MPI requires high-quality iron oxide nanoparticle tracers with tailored magnetic and surface properties to achieve its full potential. In this review, we discuss optimizing iron oxide nanoparticles’ physical, magnetic, and pharmacokinetic properties for MPI, highlighting results from our recent work in which we demonstrated tailored, biocompatible iron oxide nanoparticle tracers that provided two times better linear spatial resolution and five times better signal-to-noise ratio than Resovist. PMID:23787461

  8. Novel microwave properties and "memory effect" in magnetic nanowire array

    NASA Astrophysics Data System (ADS)

    Kou, Xiaoming

    2011-12-01

    magnetic field pulses as high as a few hundred Oe without breaking down. In the proposed EMP detector, a magnetic field sensor is required to measure the surface field of the magnetic nanowire array. MgO based magnetic tunnel junction (MTJ) is one type of magnetic field sensors. We investigated the evolution of the magnetic transport properties as a function of short annealing time in MgO based MTJ junctions. It is found that the desired sensor behavior appears in samples annealed for 17 minutes. The result can be well fitted by using the superparamagnetism theory, suggesting the formation of superparamagnetic particles in the free layer during the high temperature annealing. The control of MTJ properties with annealing time is desirable in magnetic field sensor productions.

  9. Recent advances in magnetic nanoparticles with bulk-like properties

    NASA Astrophysics Data System (ADS)

    Batlle, Xavier

    2013-03-01

    Magnetic nanoparticles (NP) are an excellent example of nanostructured materials and exhibit fascinating properties with applications in high-density recording and biomedicine. Controlling the effects of the nanostructure and surface chemistry and magnetism at the monolayer level have become relevant issues. As the size is reduced below 100 nm, deviations from bulk behavior have been attributed to finite-size effects and changes in the magnetic ordering at the surface, thus giving rise to a significant decrease in the magnetization and increase in the magnetic anisotropy. The existence of a surface spin glass-like state due to magnetic frustration has been widely suggested in ferrimagnetic NP. However, in this talk, we will show that high crystal quality magnetite Fe3-xO4 NP of about a few nanometers in diameter and coated with different organic surfactants display bulk-like structural, magnetic and electronic properties. Magnetic measurements, transmission electron microscopy, X-ray absorption and magnetic circular dichroism and Monte Carlo simulations, evidenced that none of the usual particle-like behavior is observed in high quality NP of a few nm. Consequently, the magnetic and electronic disorder phenomena typically observed in those single-phase ferrimagnetic NP should not be considered as an intrinsic effect. We also performed a real-space characterization at the sub-nanometer scale, combining scanning transmission electron microscopy, electron energy loss spectroscopy and electron magnetic chiral dichroism. For the first time, we found that the surface magnetization is as high as about 70% of that of the core. The comparison to density functional theory suggested the relevance of the strong surface bond between the Fe ions and the organic surfactant. All the foregoing demonstrates the key role of both the crystal quality and surface bond on the physical properties of ferrimagnetic NP and paves the way to the fabrication of the next generation of NP with

  10. Improvement of dose distribution in breast radiotherapy using a reversible transverse magnetic field Linac-MR unit

    SciTech Connect

    Esmaeeli, A. D.; Mahdavi, S. R.; Pouladian, M.; Bagheri, S.; Monfared, A. S.

    2014-01-15

    Purpose: To investigate the improvement in dose distribution in tangential breast radiotherapy using a reversible transverse magnetic field that maintains the same direction of Lorentz force between two fields. The investigation has a potential application in future Linac-MR units. Methods: Computed tomography images of four patients and magnetic fields of 0.25–1.5 Tesla (T) were used for Monte Carlo simulation. Two patients had intact breast while the other two had mastectomy. Simulations of planning and chest wall irradiation were similar to the actual clinical process. The direction of superior-inferior magnetic field for the medial treatment beam was reversed for the lateral beam. Results: For the ipsilateral lung and heart mean doses were reduced by a mean (range) of 45.8% (27.6%–58.6%) and 26.0% (20.2%–38.9%), respectively, depending on various treatment plan setups. The mean V{sub 20} for ipsilateral lung was reduced by 55.0% (43.6%–77.3%). In addition acceptable results were shown after simulation of 0.25 T magnetic field demonstrated in dose-volume reductions of the heart, ipsilateral lung, and noninvolved skin. Conclusions: Applying a reversible magnetic field during breast radiotherapy, not only reduces the dose to the lung and heart but also produces a sharp drop dose volume histogram for planning target volume, because of bending of the path of secondary charged particles toward the chest wall by the Lorentz force. The simulations have shown that use of the magnetic field at 1.5 T is not feasible for clinical applications due to the increase of ipsilateral chest wall skin dose in comparison to the conventional planning while 0.25 T is suitable for all patients due to dose reduction to the chest wall skin.

  11. Probing magnetic properties of ferrofluids using temperature dependent magnetic hyperthermia studies

    NASA Astrophysics Data System (ADS)

    Nemala, Humeshkar; Thakur, Jagdish; Naik, Vaman; Naik, Ratna

    2014-03-01

    Tuning the properties of magnetic nanoparticles is essential for biomedical and technological applications. An important phenomenon displayed by these nanoparticles is the generation of heat in the presence of an external oscillating magnetic field and is known as magnetic hyperthermia (MHT). The heat dissipation by the magnetic nanoparticles occurs via Neel relaxation (the flip of the internal magnetic moment of the nanoparticles) and Brownian relaxation (the physical rotation of the nanoparticles in the suspended media). Dextran coated iron oxide (Fe3O4) nanoparticles were synthesized using the co-precipitation method and characterized using XRD, TEM and DC magnetometry measurements. Roughly spherical in shape the particles have an average size of 13nm and a saturation magnetization of 65 emu/g. The MHT properties of these nanoparticles suspended in a weakly basic solution (ferrofluid) have been investigated as a function of the frequency and amplitude of magnetic field by incorporating a complete thermodynamical analysis of the experimental set-up. The heat generation is quantified using the specific power loss (SPL) and compared with the predictions of linear response theory. This analysis sheds light on important physical and magnetic properties of the nanoparticles.

  12. Magnetic structure and magnetic properties of nanocrystalline and amorphous Fe-Zr-N films

    NASA Astrophysics Data System (ADS)

    Sheftel, Elena N.; Harin, Eugene V.; Tedzhetov, Valentin A.; Kiryukhantsev-Korneev, Philipp V.; Levashov, Evgeny A.; Perov, Nikolai S.; Titova, Alexandra O.

    2016-08-01

    Data on the magnetic structure and magnetic properties of Fe-Zr-N films, which were prepared by reactive magnetron sputtering of a heated target and deposited on glass substrates, are reported. Depending on the Zr content (from 3 to 35 at%), the film compositions are characterized by Zr-to-N (at%) ratio from 0.3 to 36.5. The magnetic properties (saturation magnetization Ms, coercive field Hc) and magnetic structure (effective local magnetic anisotropy field D1/2Ha, grain size 2Rc, effective anisotropy field of stochastic domain D1/2, relative stochastic domain size RL/Rc) of the films are discussed in interrelation with their phase and structural states. The coercive field of the studied ferromagnetic nanocrystalline films was shown to obey the relationship Hc~(2Rc)6 and depends on not only the grain size but also the local magnetic anisotropy field D1/2Ha. As the grain size of ferromagnetic phase decreases, the contribution of the magnetoelastic component to the coercive field decreases. It was shown, by examples of weak ferromagnetic and superparamagnetic films with amorphous and mixed (amorphous+nanocrystalline) structures containing a nonferromagnetic phase, that the magnetic properties reflect the real structural and phase state of the films, which cannot be revealed by the X-ray diffraction analysis.

  13. Magnetic properties of NdFeB-coated rubberwood composites

    NASA Astrophysics Data System (ADS)

    Noodam, Jureeporn; Sirisathitkul, Chitnarong; Matan, Nirundorn; Rattanasakulthong, Watcharee; Jantaratana, Pongsakorn

    2013-01-01

    Magnetic properties of composites prepared by coating lacquer containing neodymium iron boron (Nd-Fe-B) powders on rubberwood were characterized by vibrating sample magnetometry (VSM), magnetic moment measurements, and attraction tests with an iron-core solenoid. The Nd-Fe-B powders were recycled from electronic wastes by the ball-milling technique. Varying the milling time from 20 to 300 min, the magnetic squareness and the coercive field of the Nd-Fe-B powders were at the minimum when the powders were milled for 130 min. It followed that the coercive field of the magnetic wood composites was increased with the milling time increasing from 130 to 300 min. For the magnetic wood composites using Nd-Fe-B obtained from the same milling time, the magnetic squareness and the coercive field were rather insensitive to the variation of Nd-Fe-B concentration in coating lacquer from 0.43 to 1.00 g/cm3. By contrast, the magnetization and magnetic moment were increased with the Nd-Fe-B concentration increasing. Furthermore, the electrical current in the solenoid required for the attraction of the magnetic wood composites was exponentially reduced with the increase in the amount of Nd-Fe-B used in the coating.

  14. Spontaneous Increase of Magnetic Flux and Chiral-Current Reversal in Bosonic Ladders: Swimming against the Tide.

    PubMed

    Greschner, S; Piraud, M; Heidrich-Meisner, F; McCulloch, I P; Schollwöck, U; Vekua, T

    2015-11-01

    The interplay between spontaneous symmetry breaking in many-body systems, the wavelike nature of quantum particles and lattice effects produces an extraordinary behavior of the chiral current of bosonic particles in the presence of a uniform magnetic flux defined on a two-leg ladder. While noninteracting as well as strongly interacting particles, stirred by the magnetic field, circulate along the system's boundary in the counterclockwise direction in the ground state, interactions stabilize vortex lattices. These states break translational symmetry, which can lead to a reversal of the circulation direction. Our predictions could readily be accessed in quantum gas experiments with existing setups or in arrays of Josephson junctions.

  15. Onset and Saturation of Ion Heating by Odd-parity Rotating-magnetic-fields in a Field-reversed Configuration

    SciTech Connect

    A.S. Landsman, S.A. Cohen, A.H. Glasser

    2005-11-01

    Heating of figure-8 ions by odd-parity rotating magnetic fields (RMFο) applied to an elongated field-reversed configuration (FRC) is investigated. The largest energy gain occurs at resonances (s ≡ ω(sub)R/ω) of the RMFο frequency, ω(sub)R, with the figure-8 orbital frequency, ω, and is proportional to s^2 for s – even resonances and to s for s – odd resonances. The threshold for the transition from regular to stochastic orbits explains both the onset and saturation of heating. The FRC magnetic geometry lowers the threshold for heating below that in the tokamak by an order of magnitude.

  16. Effects of plasma collisionality on power balance and magnetic fluctuations in the T1 reversed-field pinch

    NASA Astrophysics Data System (ADS)

    Hedin, G.; Brzozowski, J. H.; Hörling, P.; Mazur, S.; Nordlund, P.; Drake, J. R.

    1996-05-01

    The effects of plasma collisionality on power balance and magnetic fluctuations have been studied on the Extrap T1 reversed-field pinch. A characteristic minimum in loop voltage is observed as the plasma collisionality decreases. The minimum is caused by an increase in the anomalous input power and coincides with a change of scaling of the magnetic fluctuations and a rapid increase of the electron mean free path. However, the increase of anomalous input power in the low collisional regime appears to have little influence on the total amount of energy stored in the plasma.

  17. Magnetic properties and magnetic domains of Nd-Fe-B thin films

    SciTech Connect

    Chen, S. L.; Liu, W.; Zhang, Z. D.; Gunaratne, G. H.

    2008-01-15

    Anisotropic Nd-Fe-B thin films are fabricated by direct current magnetron sputtering on Si substrates heated to temperatures over a wide range. Surface morphology and magnetic domains of the Nd-Fe-B thin films prepared at different sputtering temperatures (25-600 deg. C) are observed by a scanning probe microscopy. The magnetic domains exhibit a rich variety of textures, changing from striped via maze to cloudlike as the sputtering temperature is increased. Variations in magnetic domains with substrate temperature are discussed using phase components and magnetic anisotropies of the thin films. In addition, patterns of magnetic domains are analyzed using the 'disorder functions', a set of characterizations of complex patterns with labyrinthine structures. The disorder function {delta}(1) and the structure factor {delta}k do not change appreciably until a substrate temperature of 350 deg. C, but increases significantly beyond 400 deg. C. The disorder in magnetic domains increases with increasing sputtering temperature. A simultaneous enhancement of the anisotropic c texture and the hard-magnetic properties of the thin films are observed. The significant change of the disorder function at T{sub s}=400 deg. C appears to be a precursor to the hardening of the Nd-Fe-B film. The most disordered magnetic domains of the film with the substrate temperature of 600 deg. C correspond to the optimum magnetic properties, with the maximum energy product (BH){sub max} of 22.4 MG Oe.

  18. Effect of broad properties fuel on injector performance in a reverse flow combustor

    NASA Technical Reports Server (NTRS)

    Raddlebaugh, S. M.; Norgren, C. T.

    1983-01-01

    The effect of fuel type on the performance of various fuel injectors was investigated in a reverse flow combustor. Combustor performance and emissions are documented for simplex pressure atomizing, spill flow, and airblast fuel injectors using a broad properties fuel and compared with performance using Jet A fuel. Test conditions simulated a range of flight conditions including sea level take off, low and high altitude cruise, as well as a parametric evaluation of the effect of increased combustor loading. The baseline simplex injector produced higher emission levels with corresponding lower combustion efficiency with the broad properties fuel. There was little or not loss in performance by the two advanced concept injectors with the broad properties fuel. The airblast injector proved to be especially insensitive to fuel type.

  19. Micromagnetic simulation of the orientation dependence of grain boundary properties on the coercivity of Nd-Fe-B sintered magnets

    NASA Astrophysics Data System (ADS)

    Fujisaki, Jun; Furuya, Atsushi; Uehara, Yuji; Shimizu, Koichi; Ataka, Tadashi; Tanaka, Tomohiro; Oshima, Hirotaka; Ohkubo, Tadakatsu; Hirosawa, Satoshi; Hono, Kazuhiro

    2016-05-01

    This paper is focused on the micromagnetic simulation study about the orientation dependence of grain boundary properties on the coercivity of polycrystalline Nd-Fe-B sintered magnets. A multigrain object with a large number of meshes is introduced to analyze such anisotropic grain boundaries and the simulation is performed by combining the finite element method and the parallel computing. When the grain boundary phase parallel to the c-plane is less ferromagnetic the process of the magnetization reversal changes and the coercivity of the multigrain object increases. The simulations with various magnetic properties of the grain boundary phases are executed to search for the way to enhance the coercivity of polycrystalline Nd-Fe-B sintered magnets.

  20. Coercivity, microstructure and magnetization reversal mechanism in TiNi-doped L10 FePt thin films

    NASA Astrophysics Data System (ADS)

    Zhang, Yongmei; Li, Xiaohong; Jing, Jingjing; Zhang, Xiangyi; Zhao, Yuhong

    2016-06-01

    Controlling coercivity and understanding how it is affected by the microstructure are of essential importance for practical application of FePt thin films as a recording media. In this study, the small size of ordered domain, lower coercivity and weak intergranular exchange coupling interaction in TiNi-doped L10 FePt thin films are obtained. The TiNi additions maybe diffuse out of the FePt lattice into FePt grain boundaries, which separate FePt grains. The doping in grain boundary provides the nucleation center of reversed domain, which leads both nucleation-type and pinning-type mechanism to coexist in magnetization reversal processes for TiNi-doped FePt thin films. The decrease of anisotropy constant and nucleation field of reversed domain provides an explanation for the coercivity reduction of FePt thin films after TiNi doping.

  1. GEMAS: Unmixing magnetic properties of European agricultural soil

    NASA Astrophysics Data System (ADS)

    Fabian, Karl; Reimann, Clemens; Kuzina, Dilyara; Kosareva, Lina; Fattakhova, Leysan; Nurgaliev, Danis

    2016-04-01

    High resolution magnetic measurements provide new methods for world-wide characterization and monitoring of agricultural soil which is essential for quantifying geologic and human impact on the critical zone environment and consequences of climatic change, for planning economic and ecological land use, and for forensic applications. Hysteresis measurements of all Ap samples from the GEMAS survey yield a comprehensive overview of mineral magnetic properties in European agricultural soil on a continental scale. Low (460 Hz), and high frequency (4600 Hz) magnetic susceptibility k were measured using a Bartington MS2B sensor. Hysteresis properties were determined by a J-coercivity spectrometer, built at the paleomagnetic laboratory of Kazan University, providing for each sample a modified hysteresis loop, backfield curve, acquisition curve of isothermal remanent magnetization, and a viscous IRM decay spectrum. Each measurement set is obtained in a single run from zero field up to 1.5 T and back to -1.5 T. The resulting data are used to create the first continental-scale maps of magnetic soil parameters. Because the GEMAS geochemical atlas contains a comprehensive set of geochemical data for the same soil samples, the new data can be used to map magnetic parameters in relation to chemical and geological parameters. The data set also provides a unique opportunity to analyze the magnetic mineral fraction of the soil samples by unmixing their IRM acquisition curves. The endmember coefficients are interpreted by linear inversion for other magnetic, physical and chemical properties which results in an unprecedented and detailed view of the mineral magnetic composition of European agricultural soils.

  2. Low Temperature Crystal Structure and Magnetic Properties of RAl2

    SciTech Connect

    Pathak, Arjun K.; Paudyal, Durga; Gschneidner, Karl A.; Pecharsky, Vitalij K.

    2014-01-08

    Low temperature crystal structure and magnetic properties of RAl2 (R = Pr and Nd) have been studied using temperature dependent powder x-ray diffraction, magnetization, and heat capacity measurements. Unlike PrAl2, NdAl2 retains cubic MgCu2-type structure from room temperature down to 5 K, which is also confirmed from first principles electronic structure calculations. The magnetization measurements show both PrAl2 and NdAl2 order ferromagnetically at TC = 32 K and 77 K, respectively. However, the magnetization measurements show the former is a hard ferromagnet compared to the latter which is a soft ferromagnetic material. The magnetic entropy change obtained from heat capacity measurements at ΔH = 30 kOe for PrAl2 and NdAl2 are 3.15 J mol-1 K-1 and 1.18 J mol-1 K-1, respectively.

  3. Microstructure and Magnetic Properties of Bulk Nanocrystalline MnAl

    SciTech Connect

    Chaturvedi, A; Yaqub, R; Baker, I

    2014-01-22

    MnAl is a promising rare-earth free permanent magnet for technological use. We have examined the effects of consolidation by back-pressure, assisted equal channel angular extrusion processing on mechanically-milled, gas-atomized Mn-46% at. Al powder. X-ray diffraction showed both that the extruded rod consisted mostly of metastable tau phase, with some of the equilibrium gamma(2) and beta phases, and that it largely retained the as-milled nanostructure. Magnetic measurements show a coercivity of <= 4.4 kOe and a magnetization at 10 kOe of <= 40 emu/g. In addition, extrusions exhibit greater than 95% of the theoretical density. This study opens a new window in the area of bulk MnAl magnets with improved magnetic properties for technological use.

  4. Dust properties and magnetic field geometry towards LDN 1570

    NASA Astrophysics Data System (ADS)

    Eswaraiah, C.; Maheswar, G.; Pandey, A. K.

    2015-03-01

    We have performed both optical linear polarimetric and photometric observations of an isolated dark globule LDN 1570 aim to study the dust polarizing and extinction properties and to map the magnetic field geometry so as to understand not only the importance of magnetic fields in formation and evolution of clouds but also the correlation of the inferred magnetic field structure with the cloud structure and its dynamics. Dust size indicators (R V and λ max ) reveal for the presence of slightly bigger dust grains towards the cloud region. The inferred magnetic field geometry, which closely follows the cloud structure revealed by Herschel images, suggest that the cloud could have been formed due to converging material flows along the magnetic field lines.

  5. Structure, synthetic methods, magnetic properties and biomedical applications of ferrofluids.

    PubMed

    Shokrollahi, H

    2013-07-01

    This paper is aimed at conducting a survey of the synthetic methods and magnetic properties of nanoparticles as ferrofluids used in biomedicine. As compared with other works in the field, the distinctive feature of the current work is the systematic study of recent advances in ferrofluids utilized in hyperthermia and magnetic resonance imaging (MRI). The most important feature for application of ferrofluids is super-paramagnetic behavior of magnetic cores with relatively high saturation magnetization. Although Fe3O4 nanoparticles have traditionally been used in medicine; the modified Mn-ferrite has recently received special attention due to its higher saturation magnetization and r2-relaxivity as a contrast agent in MRI. Co-ferrite nanoparticles are also good candidates for hyperthermia treatment because of their high coercivity and magnetocrystalline anisotropy. The thermal decomposition and hydrothermal methods are good candidates for obtaining appropriate super-paramagnetic particles. PMID:23623058

  6. Single crystal Processing and magnetic properties of gadolinium nickel

    SciTech Connect

    Shreve, Andrew John

    2012-01-01

    GdNi is a rare earth intermetallic material that exhibits very interesting magnetic properties. Spontaneous magnetostriction occurs in GdNi at T{sub C}, on the order of 8000ppm strain along the c-axis and only until very recently the mechanism causing this giant magnetostriction was not understood. In order to learn more about the electronic and magnetic structure of GdNi, single crystals are required for anisotropic magnetic property measurements. Single crystal processing is quite challenging for GdNi though since the rare-earth transition-metal composition yields a very reactive intermetallic compound. Many crystal growth methods are pursued in this study including crucible free methods, precipitation growths, and specially developed Bridgman crucibles. A plasma-sprayed Gd2O3 W-backed Bridgman crucible was found to be the best means of GdNi single crystal processing. With a source of high-quality single crystals, many magnetization measurements were collected to reveal the magnetic structure of GdNi. Heat capacity and the magnetocaloric effect are also measured on a single crystal sample. The result is a thorough report on high quality single crystal processing and the magnetic properties of GdNi.

  7. Particle size dependent rheological property in magnetic fluid

    NASA Astrophysics Data System (ADS)

    Wu, Jie; Pei, Lei; Xuan, Shouhu; Yan, Qifan; Gong, Xinglong

    2016-06-01

    The influence of the particle size on the rheological property of magnetic fluid was studied both by the experimental and computer simulation methods. Firstly, the magnetic fluids were prepared by dispersing Fe3O4 nanospheres with size varied from 40 nm to 100 nm and 200 nm in the solution. Then, the rheological properties were investigated and it was found that the relative magnetorheological effects increased with increasing the particle size. Finally, the molecular dynamic simulation was used to analyze the mechanical characteristics of the magnetic fluid and the chain-like model agreed well with the experimental result. The authentic chain-like structure observed by a microscope agreed with the simulation results. The three particles composed of the similar cluster nanostructure, thus they exhibited similar magnetic property. To this end, the unique assembling microstructures was the origination of the mechanical difference. And it was found that the higher MR (magnetorheological) effects of the large particle based magnetic fluid was originated from the stronger assembling microstructure under the applying magnetic field.

  8. Magnetic Nanoparticles: Surface Effects and Properties Related to Biomedicine Applications

    PubMed Central

    Issa, Bashar; Obaidat, Ihab M.; Albiss, Borhan A.; Haik, Yousef

    2013-01-01

    Due to finite size effects, such as the high surface-to-volume ratio and different crystal structures, magnetic nanoparticles are found to exhibit interesting and considerably different magnetic properties than those found in their corresponding bulk materials. These nanoparticles can be synthesized in several ways (e.g., chemical and physical) with controllable sizes enabling their comparison to biological organisms from cells (10–100 μm), viruses, genes, down to proteins (3–50 nm). The optimization of the nanoparticles’ size, size distribution, agglomeration, coating, and shapes along with their unique magnetic properties prompted the application of nanoparticles of this type in diverse fields. Biomedicine is one of these fields where intensive research is currently being conducted. In this review, we will discuss the magnetic properties of nanoparticles which are directly related to their applications in biomedicine. We will focus mainly on surface effects and ferrite nanoparticles, and on one diagnostic application of magnetic nanoparticles as magnetic resonance imaging contrast agents. PMID:24232575

  9. Control of Magnetic Properties of Carbon Nanotubes Filled with Iron

    NASA Astrophysics Data System (ADS)

    Sato, Hideki; Nagata, Atsushi; Kubonaka, Nobuo; Fujiwara, Yuji

    2013-11-01

    Carbon nanotubes (CNTs) filled with iron nanowires show high coercivity owing to their shape anisotropy originating from the high-aspect-ratio shapes of the iron nanowires. In this study, CNTs filled with iron were prepared by the thermal chemical vapor deposition (T-CVD) method using ferrocene as a precursor, and the magnetic properties of the synthesized CNTs were examined in detail. It was found that the CVD temperature and the amount of the ferrocene introduced into the CVD reactor influence the amount of CNT growth and the magnetic properties. The high coercivity of approximately 1.6 kOe or higher was obtained under certain CVD conditions. The selected-area electron diffraction analysis showed that the magnetic properties of the CNTs filled with iron are determined by the crystal structure (α-Fe or Fe3C) of the iron nanowires, which can be controlled by the amount of the ferrocene supplied during CVD.

  10. Electronic, magnetic and transport properties of rare-earth monopnictides.

    PubMed

    Duan, Chun-Gang; Sabirianov, R F; Mei, W N; Dowben, P A; Jaswal, S S; Tsymbal, E Y

    2007-08-01

    The electronic structures and magnetic properties of many rare-earth monopnictides are reviewed in this article. Possible candidate materials for spintronics devices from the rare-earth monopnictide family, i.e. high polarization (nominally half-metallic) ferromagnets and antiferromagnets, are identified. We attempt to provide a unified picture of the electronic properties of these strongly correlated systems. The relative merits of several ab initio theoretical methods, useful in the study of the rare-earth monopnictides, are discussed. We present our current understanding of the possible half-metallicity, semiconductor-metal transitions, and magnetic orderings in the rare-earth monopnictides. Finally, we propose some potential strategies to improve the magnetic and electronic properties of these candidate materials for spintronics devices. PMID:21694120

  11. Magnetic properties of superparamagnetic nanoparticles loaded into silicon nanotubes

    NASA Astrophysics Data System (ADS)

    Granitzer, Petra; Rumpf, Klemens; Gonzalez, Roberto; Coffer, Jeffery; Reissner, Michael

    2014-08-01

    In this work, the magnetic properties of silicon nanotubes (SiNTs) filled with Fe3O4 nanoparticles (NPs) are investigated. SiNTs with different wall thicknesses of 10 and 70 nm and an inner diameter of approximately 50 nm are prepared and filled with superparamagnetic iron oxide nanoparticles of 4 and 10 nm in diameter. The infiltration process of the NPs into the tubes and dependence on the wall-thickness is described. Furthermore, data from magnetization measurements of the nanocomposite systems are analyzed in terms of iron oxide nanoparticle size dependence. Such biocompatible nanocomposites have potential merit in the field of magnetically guided drug delivery vehicles.

  12. Magnetic properties of lithium-transition metal orthophosphates

    NASA Astrophysics Data System (ADS)

    Semkin, Mikhail; Choi, Ki-Young; Sim, Hasung; Urusova, Natali; Volegov, Aleksey; Barykina, Julia; Kellerman, Dina; Park, Je-Geun; Pirogov, Alexander

    2016-09-01

    Magnetic properties of the lithium-transition metal orthophosphates LiNiPO4, LiNi0.9Co0.1PO4, LiNi0.9Mn0.1PO4 and LiMnPO4 single crystals have been studied. Temperature behavior of a susceptibility against a type of 3d-transition ion was analyzed. Anomalous behavior is observed over narrow temperature region near Neel point. This is caused by a commensurate-incommensurate magnetic phase transition in pure LiNiPO4, Co- and Mn-doped samples. Using Curie-Weiss model we calculated magnetic constants.

  13. The Reversed Role of Magnets in St. Louis: Implications for Black Student Outcomes

    ERIC Educational Resources Information Center

    Grooms, Ain A.; Williams, Sheneka M.

    2015-01-01

    Magnet schools were originally created to attract a diverse student population. Using data from the 23 magnet schools in St. Louis, this longitudinal study is twofold: first, to review the performance outcomes of the magnet schools across a 5-year period, between 2005-2006 and 2009-2010, and second, to examine whether the magnet schools are…

  14. Left ventricular reverse remodeling after transcatheter aortic valve implantation: a cardiovascular magnetic resonance study

    PubMed Central

    2013-01-01

    Background In patients with severe aortic stenosis, left ventricular hypertrophy is associated with increased myocardial stiffness and dysfunction linked to cardiac morbidity and mortality. We aimed at systematically investigating the degree of left ventricular mass regression and changes in left ventricular function six months after transcatheter aortic valve implantation (TAVI) by cardiovascular magnetic resonance (CMR). Methods Left ventricular mass indexed to body surface area (LVMi), end diastolic volume indexed to body surface area (LVEDVi), left ventricular ejection fraction (LVEF) and stroke volume (SV) were investigated by CMR before and six months after TAVI in patients with severe aortic stenosis and contraindications for surgical aortic valve replacement. Results Twenty-sevent patients had paired CMR at baseline and at 6-month follow-up (N=27), with a mean age of 80.7±5.2 years. LVMi decreased from 84.5±25.2 g/m2 at baseline to 69.4±18.4 g/m2 at six months follow-up (P<0.001). LVEDVi (87.2±30.1 ml /m2vs 86.4±22.3 ml/m2; P=0.84), LVEF (61.5±14.5% vs 65.1±7.2%, P=0.08) and SV (89.2±22 ml vs 94.7±26.5 ml; P=0.25) did not change significantly. Conclusions Based on CMR, significant left ventricular reverse remodeling occurs six months after TAVI. PMID:23692630

  15. Gold Nanorod-pNIPAM Hybrids with Reversible Plasmon Coupling: Synthesis, Modeling, and SERS Properties.

    PubMed

    Fernández-López, Cristina; Polavarapu, Lakshminarayana; Solís, Diego M; Taboada, José M; Obelleiro, Fernando; Contreras-Cáceres, Rafael; Pastoriza-Santos, Isabel; Pérez-Juste, Jorge

    2015-06-17

    The thermoresponsive optical properties of Au nanorod-doped poly(N-isopropylacrylamide) (Au NR-pNIPAM) microgels with different Au NR payloads and aspect ratios are presented. Since the volume phase transition of pure pNIPAM microgels is reversible, the optical response reversibility of Au NR-pNIPAM hybrids is systematically analyzed. Besides, extinction cross-section and near-field enhancement simulations for Au NR-microgel hybrids are performed using a new numerical method based on the surface integral equation method of moments formulation (M3 solver). Additionally, the Au NR-microgel hybrid systems are expected to serve as excellent broadband surface-enhanced Raman scattering (SERS) substrates due to the temperature-controlled formation of hot spots and the tunable optical properties. The optical enhancing properties related to SERS are tested with three laser lines, evidencing excitation wavelength-dependent efficiency that can be easily controlled by either the aspect ratio (length/width) of the assembled Au NR or by the Au NR payload per microgel. Finally, the SERS efficiency of the prepared Au NR-pNIPAM hybrids is found to be stable for months.

  16. Gold Nanorod-pNIPAM Hybrids with Reversible Plasmon Coupling: Synthesis, Modeling, and SERS Properties.

    PubMed

    Fernández-López, Cristina; Polavarapu, Lakshminarayana; Solís, Diego M; Taboada, José M; Obelleiro, Fernando; Contreras-Cáceres, Rafael; Pastoriza-Santos, Isabel; Pérez-Juste, Jorge

    2015-06-17

    The thermoresponsive optical properties of Au nanorod-doped poly(N-isopropylacrylamide) (Au NR-pNIPAM) microgels with different Au NR payloads and aspect ratios are presented. Since the volume phase transition of pure pNIPAM microgels is reversible, the optical response reversibility of Au NR-pNIPAM hybrids is systematically analyzed. Besides, extinction cross-section and near-field enhancement simulations for Au NR-microgel hybrids are performed using a new numerical method based on the surface integral equation method of moments formulation (M3 solver). Additionally, the Au NR-microgel hybrid systems are expected to serve as excellent broadband surface-enhanced Raman scattering (SERS) substrates due to the temperature-controlled formation of hot spots and the tunable optical properties. The optical enhancing properties related to SERS are tested with three laser lines, evidencing excitation wavelength-dependent efficiency that can be easily controlled by either the aspect ratio (length/width) of the assembled Au NR or by the Au NR payload per microgel. Finally, the SERS efficiency of the prepared Au NR-pNIPAM hybrids is found to be stable for months. PMID:25850108

  17. Composite Materials with Magnetically Aligned Carbon Nanoparticles Having Enhanced Electrical Properties and Methods of Preparation

    NASA Technical Reports Server (NTRS)

    Hong, Haiping (Inventor); Peterson, G.P. (Bud) (Inventor); Salem, David R. (Inventor)

    2016-01-01

    Magnetically aligned carbon nanoparticle composites have enhanced electrical properties. The composites comprise carbon nanoparticles, a host material, magnetically sensitive nanoparticles and a surfactant. In addition to enhanced electrical properties, the composites can have enhanced mechanical and thermal properties.

  18. Estimation of hydrothermal deposits location from magnetization distribution and magnetic properties in the North Fiji Basin

    NASA Astrophysics Data System (ADS)

    Choi, S.; Kim, C.; Park, C.; Kim, H.

    2013-12-01

    The North Fiji Basin is belong to one of the youngest basins of back-arc basins in the southwest Pacific (from 12 Ma ago). We performed the marine magnetic and the bathymetry survey in the North Fiji Basin for finding the submarine hydrothermal deposits in April 2012. We acquired magnetic and bathymetry datasets by using Multi-Beam Echo Sounder EM120 (Kongsberg Co.) and Overhouser Proton Magnetometer SeaSPY (Marine Magnetics Co.). We conducted the data processing to obtain detailed seabed topography, magnetic anomaly, reduce to the pole(RTP), analytic signal and magnetization. The study areas composed of the two areas(KF-1(longitude : 173.5 ~ 173.7 and latitude : -16.2 ~ -16.5) and KF-3(longitude : 173.4 ~ 173.6 and latitude : -18.7 ~ -19.1)) in Central Spreading Ridge(CSR) and one area(KF-2(longitude : 173.7 ~ 174 and latitude : -16.8 ~ -17.2)) in Triple Junction(TJ). The seabed topography of KF-1 existed thin horst in two grabens that trends NW-SE direction. The magnetic properties of KF-1 showed high magnetic anomalies in center part and magnetic lineament structure of trending E-W direction. In the magnetization distribution of KF-1, the low magnetization zone matches well with a strong analytic signal in the northeastern part. KF-2 area has TJ. The seabed topography formed like Y-shape and showed a high feature in the center of TJ. The magnetic properties of KF-2 displayed high magnetic anomalies in N-S spreading ridge center and northwestern part. In the magnetization distribution of KF-2, the low magnetization zone matches well with a strong analytic signal in the northeastern part. The seabed topography of KF-3 presented a flat and high topography like dome structure at center axis and some seamounts scattered around the axis. The magnetic properties of KF-3 showed high magnetic anomalies in N-S spreading ridge center part. In the magnetization of KF-2, the low magnetization zone mismatches to strong analytic signal in this area. The difference of KF-3

  19. Influence of reverse bias on the LEDs properties used as photo-detectors in VLC systems

    NASA Astrophysics Data System (ADS)

    Kowalczyk, Marcin; Siuzdak, Jerzy

    2015-09-01

    Continuous increasing share of light emitting diodes (LEDs) in a lighting market, which we observe during the last couple years, opens new possibilities. Especially, when we talk about practical realization the concept of visible light communications (VLC), which gains on popularity recently. The VLC concept presupposes utilization of illumination systems for a purpose of data transmission. It means, the emitters, in this case the LEDs, will not of a light source only, but also the data transmitters. Currently, most of the conducted researches in this area is concentrated on achievement of effective transmission methods. It means a transmission only in one direction. This is not enough, when we talk about the fully functional transmission system. Ensuring of feedback transmission channel is a necessary also. One of the ideas, which was postulated by authors of this article, is using for this purpose the LEDs in a double role. A utilization of LEDs as photo-detectors requires a reverse polarization, in contrast to a forward bias, which has a place when they work as light emitters. Ensuring of proper polarization get significant meaning. The article presents the investigations results on the influence of reverse bias on photo-receiving properties of LEDs used as light detectors. The conducted research proved that an improvement of sensitivity and bandwidth parameters are possible by application of appropriate value of the reverse voltage in a receiver.

  20. Magnetic properties of heat treated bacterial ferrihydrite nanoparticles

    NASA Astrophysics Data System (ADS)

    Balaev, D. A.; Krasikov, A. A.; Dubrovskiy, A. A.; Popkov, S. I.; Stolyar, S. V.; Bayukov, O. A.; Iskhakov, R. S.; Ladygina, V. P.; Yaroslavtsev, R. N.

    2016-07-01

    The magnetic properties of ferrihydrite nanoparticles, which are products of vital functions of Klebsiella oxitoca bacteria, have been studied. The initial powder containing the nanoparticles in an organic shell was subjected to low-temperature (T=160 °C) heat treatment for up to 240 h. The bacterial ferrihydrite particles exhibit a superparamagnetic behavior. Their characteristic blocking temperature increases from 26 to 80 K with the heat treatment. Analysis of the magnetization curves with regard to the magnetic moment distribution function and antiferromagnetic contribution shows that the low-temperature heat treatment enhances the average magnetic moment of a particle; i.e., the nanoparticles coarsen, probably due to their partial agglomeration during heat treatment. It was established that the blocking temperature nonlinearly depends on the particle volume. Therefore, a model was proposed that takes into account both the bulk and surface magnetic anisotropy. Using this model, the bulk and surface magnetic anisotropy constants KV≈1.7×105 erg/cm3 and KS≈0.055 erg/cm2 have been determined. The effect of the surface magnetic anisotropy of ferrihydrite nanoparticles on the observed magnetic hysteresis loops is discussed.

  1. Magnetic properties and scale-up of nanostructured cobalt carbide permanent magnetic powders

    SciTech Connect

    Zamanpour, Mehdi Bennett, Steven; Taheri, Parisa; Chen, Yajie; Harris, Vincent G.

    2014-05-07

    Co{sub x}C magnetic nanoparticles were successfully synthesized via a modified polyol process without using a rare-earth catalyst during the synthesis process. The present results show admixtures of Co{sub 2}C and Co{sub 3}C phases possessing magnetization values exceeding 45 emu/g and coercivity values exceeding 2.3 kOe at room temperature. Moreover, these experiments have illuminated the important role of surfactants, reaction temperature, and reaction duration on the crystallographic structure and magnetic properties of Co{sub x}C, while tetraethylene glycol was employed as a reducing agent. The role of the ratios of Co{sub 2}C and Co{sub 3}C phases in the admixture magnetic properties is discussed. The crystallographic structure and particle size of the Co{sub x}C nanoparticles were characterized by X-ray diffractometry and scanning electron microscopy. Vibrating sample magnetometry was used to determine magnetic properties. Scale-up of synthesis to more than 5 g per batch was demonstrated with no significant degradation of magnetic properties.

  2. Control of Magnetic Properties Across Metal to Insulator Transitions

    NASA Astrophysics Data System (ADS)

    de La Venta, Jose

    2013-03-01

    Controlling the magnetic properties of ferromagnetic (FM) thin films without magnetic fields is an on-going challenge in condensed matter physics with multiple technological implications. External stimuli and proximity effects are the most used methods to control the magnetic properties. An interesting possibility arises when ferromagnets are in proximity to materials that undergo a metal-insulator (MIT) and structural phase transition (SPT). The stress associated with the structural changes produces a magnetoelastic anisotropy in proximity coupled ferromagnetic films that allows controlling the magnetic properties without magnetic fields. Canonical examples of materials that undergo MIT and SPT are the vanadium oxides (VO2 and V2O3) . VO2 undergoes a metal/rutile to an insulator/monoclinic phase transition at 340 K. In V2O3 the transition at 160 K is from a metallic/rhombohedral to an insulating/ monoclinic phase. We have investigated the magnetic properties of different combinations of ferromagnetic (Ni, Co and Fe) and vanadium oxide thin films. The (0.32%) volume expansion in VO2 or the (1.4%) volume decrease in V2O3 across the MIT produces an interfacial stress in the FM overlayer. We show that the coercivities and magnetizations of the ferromagnetic films grown on vanadium oxides are strongly affected by the phase transition. The changes in coercivity can be as large as 168% and occur in a very narrow temperature interval. These effects can be controlled by the thickness and deposition conditions of the different ferromagnetic films. For VO2/Ni bilayers the large change in the coercivity occurring above room temperature opens the possibilities for technological applications. Work done in collaboration with Siming Wang, J. G. Ramirez, and Ivan K. Schuller. Funded by the US DoE, Office of Basic Energy Sciences, under Award FG03-87ER-45332 and the Air Force Office of Scientific Research No. FA9550-12-1-0381.

  3. Magnetic properties of square Py nanowires: Irradiation dose and geometry dependence

    SciTech Connect

    Ehrmann, A.; Blachowicz, T.; Komraus, S.; Nees, M.-K.; Jakobs, P.-J.; Leiste, H.; Mathes, M.; Schaarschmidt, M.

    2015-05-07

    Arrays of ferromagnetic patterned nanostructures with single particle lateral dimensions between 160 nm and 400 nm were created by electron-beam lithography. The fourfold particles with rectangular-shaped walls around a square open area were produced from permalloy. Their magnetic properties were measured using the longitudinal magneto-optical Kerr effect. The article reports about the angle-dependent coercive fields and the influence of the e-beam radiation dose on sample shapes. It is shown that a broad range of radiation dose intensities enables reliable creation of nanostructures with parameters relevant for the desired magnetization reversal scenario. The experimental results are finally compared with micromagnetic simulations to explain the findings.

  4. Magnetic and structural properties of MnBi multilayered thin films

    SciTech Connect

    Hozumi, T.; LeClair, P.; Mankey, G.; Mewes, C.; Suzuki, T.; Sepehri-Amin, H.; Hono, K.

    2014-05-07

    Magnetic and structural properties of MnBi films with thicknesses up to 50 nm were investigated. Thin films of the MnBi LTP (Low Temperature Phase) were fabricated onto silica-glass substrates by sputter-deposition of Bi/Mn multilayer, followed by a subsequent annealing at about 550 °C for 30 min. Coercivity of such thin films is higher than 15 kOe, even though the film thickness is about 10 nm. These thin films show the preferential growth of c-axis of the LTP along the film normal. Moreover, high resolution transmission electron microscopy indicates that the LTP regions of 30–50 nm in size are physically isolated by Bi. The magnetization reversal mechanism of such a LTP region is mainly governed by a coherent rotation mode based on the δM curve measurement.

  5. Size-dependent structure and magnetic properties of DyMnO{sub 3} nanoparticles

    SciTech Connect

    Cai, Xuan; Shi, Lei Zhou, Shiming; Zhao, Jiyin; Guo, Yuqiao; Wang, Cailin

    2014-09-14

    The structure and magnetic properties of orthorhombic DyMnO{sub 3} nanoparticles with different particle sizes are investigated in this paper. With decreasing particle size, all the lattice parameters a, b, and c gradually decrease, whereas the orthorhombic distortion increases. Magnetic measurements reveal that the antiferromagnetic interaction of Mn ions is weakened due to the decrease in Mn-O-Mn bond angle. Above a critical field H*, DyMnO{sub 3} undergoes a field-induced metamagnetic transition at 4 K, which is related to the spin reversal of Dy moments. The critical field H* increases monotonically with size reduction, indicating an enhancement of the antiferromagnetic interaction of Dy ions due to the decreased distance between rare earth ions. The magnetization at 4 K and 5 T, i.e., M(4 K, 5 T) shows a non-monotonic variation with particle size d, i.e., M(4 K, 5 T) initially increases with size reduction but decreases again for d < 68 nm. A modified core-shell model, in which the ferromagnetic ordering (Dy magnetic structure) and antiferromagnetic ordering (Mn magnetic structure) coexist in the core, is proposed to explain this behavior.

  6. Microstructure and magnetic properties of soft magnetic powder cores of amorphous and nanocrystalline alloys

    NASA Astrophysics Data System (ADS)

    Liu, Yapi; Yi, Yide; Shao, Wei; Shao, Yanfang

    2013-03-01

    With the development of modern ferromagnetic technology, soft magnetic powder cores (MPCs) of amorphous and nanocrystalline alloys have been intensively studied for their excellent soft magnetic properties such as high flux density, low coercivity and reduced core loss due to amorphous state and nanocrystalline grains of 10-20 nm dispersed in a residual amorphous matrix. In this paper, the microstructures and soft magnetic properties, i.e., maximum magnetic induction Bm, effective permeability μe, DC-bias properties and volume power losses PCV of MPCs made from amorphous powder of gas atomization and nanocrystalline powder of pulverized melt-spun ribbon were investigated and also compared on the basis of the same level of μe. It is found that μe of both kinds of MPC keeps unchanged up to 1 MHz. The amorphous MPC has lower PCV at lower frequency range, while the nanocrystalline MPC has lower PCV at high frequency range instead. Also, the nanocrystalline MPC has better DC-bias property. Moreover, the DC magnetic properties and the changes of PCV of both MPCs with frequency and flux density are also studied. Furthermore, the electromagnetic characteristics, the microstructures and the mechanisms accounting for these phenomena of both MPCs are also discussed.

  7. Thermo-electromagnetic properties of a magnetically shielded superconductor strip: theoretical foundations and numerical simulations

    NASA Astrophysics Data System (ADS)

    Ma, G. T.; Rauh, H.

    2013-10-01

    Numerical simulations of thermo-electromagnetic properties of a thin type-II superconductor strip surrounded by open cavity soft-magnetic shields and exposed to an oscillating transverse magnetic field are performed by resorting to the quasistatic approximation of a vector potential approach in conjunction with the classical description of conduction of heat. The underlying definition of the superconducting constituent makes use of an extended ‘smoothed’ Bean model of the critical state, which includes the field and temperature dependence of the induced supercurrent as well. The delineation of the magnetic shields exploits the reversible-paramagnet approximation in the Langevin form, as appropriate for magnetizations with narrow Z-type loops, and considers induced eddy currents too. The coolant is envisaged as acting like a bath that instantly takes away surplus heat. Based on the Jacobian-free Newton-Krylov approach and the backward Euler scheme, the numerical analysis at hand is tailored to the problem of a high width/thickness aspect ratio of the superconductor strip. Assigning representative materials characteristics and conditions of the applied magnetic field, the main findings for a practically relevant magnet configuration include: (i) an overall rise of the maximum temperature of the superconductor strip tending to saturation in a superconducting thermo-electromagnetic steady state above the operating temperature, magnetic shielding lending increased stability and smoothing the temperature profile along the width of the superconductor strip; (ii) a washing out of the profile of the magnetic induction and a lowering of its strength, a relaxation of the profile of the supercurrent density and an increase of its strength, a tightening of the power loss density and a reduction of its strength, all inside the superconductor strip. The hysteretic ac loss suffered by the superconductor strip is seen to be cut back or, at most, to converge on that of an

  8. Magnetic Properties of Different-Aged Chernozemic Soils

    NASA Astrophysics Data System (ADS)

    Fattakhova, Leysan; Shinkarev, Alexandr; Kosareva, Lina; Nourgaliev, Danis; Shinkarev, Aleksey; Kondrashina, Yuliya

    2016-04-01

    We investigated the magnetic properties and degree of mineral weathering in profiles of different-aged chernozemic soils derived from a uniform parent material. In this work, layer samples of virgin leached chernozem and chernozemic soils formed on the mound of archaeological earthy monument were used. The characterization of the magnetic properties was carried out on the data of the magnetometry and differential thermomagnetic analysis. The evaluation of the weathering degree was carried out on a loss on ignition, cation exchange capacity and X-ray phase analysis on the data of the original soil samples and samples of the heavy fraction of minerals. It was found that the magnetic susceptibility enhancement in humus profiles of newly formed chernozemic soils lagged significantly behind the organic matter content enhancement. This phenomenon is associated with differences in kinetic parameters of humus formation and structural and compositional transformation of the parent material. It is not enough time of 800-900 years to form a relatively "mature" magnetic profile. These findings are well consistent with the chemical kinetic model (Boyle et al., 2010) linking the formation of the soils magnetic susceptibility with the weathering of primary Fe silicate minerals. Different-aged chernozemic soils are at the first stage of formation of a magnetic profile when it is occur an active production of secondary ferrimagnetic minerals from Fe2+ released by primary minerals.

  9. Monotonic and fatigue properties of kenaf /glass hybrid composites under fully reversed cyclic loading

    NASA Astrophysics Data System (ADS)

    Sharba, M. J.; Leman, Z.; Sultan, M. T. H.; Ishak, M. R.; Hanim, M. A. A.

    2015-12-01

    The aim of this work is to investigate the effect of hybridization of kenaf-glass fibers reinforced unsaturated polyester on fatigue life. Three types of composites were fabricated using hands lay-up method, namely, kenaf, glass, and hybrid composites with 30% of weight fraction, the hybrid was mixed with a ratio of kenaf: glass 10:20. Monotonic tests were achieved (Tensile and compression) to determine the fatigue stress levels. Fully reversed fatigue loading was conducted with a stress ratio of -1 and stress levels 55-85% of the ultimate static stresses, all tests were conducted at 10 Hz of frequency. The results proof a positive hybrid composite; also agree with the rule of mixture that can predict the final composite properties. Moreover, it's been observed an improvement in overall mechanical properties of hybrid compared to individual ones.

  10. White-Light-Emitting Lanthanide Metallogels with Tunable Luminescence and Reversible Stimuli-Responsive Properties.

    PubMed

    Chen, Pangkuan; Li, Qiaochu; Grindy, Scott; Holten-Andersen, Niels

    2015-09-16

    We have developed model light-emitting metallogels functionalized with lanthanide metal-ligand coordination complexes via a terpyridyl-end-capped four-arm poly(ethylene glycol) polymer. The optical properties of these highly luminescent polymer networks are readily modulated over a wide spectrum, including white-light emission, simply by tuning of the lanthanide metal ion stoichiometry. Furthermore, the dynamic nature of the Ln-N coordination bonding leads to a broad variety of reversible stimuli-responsive properties (mechano-, vapo-, thermo-, and chemochromism) of both sol-gel systems and solid thin films. The versatile functional performance combined with the ease of assembly suggests that this lanthanide coordination polymer design approach offers a robust pathway for future engineering of multi-stimuli-responsive polymer materials. PMID:26301493

  11. Tailoring magnetic properties in arrays of pulse-electrodeposited Co nanowires: The role of Cu additive

    NASA Astrophysics Data System (ADS)

    Esmaeili, A.; Almasi Kashi, M.; Ramazani, A.; Montazer, A. H.

    2016-01-01

    In this study, we aim to report the role of Cu additive in arrays of pulse-electrodeposited Co nanowires (NWs) with diameters from 30 to 75 nm, embedded in porous aluminum oxide templates. This features the role of Cu additive in composition and crystalline characteristics as well as in the magnetic properties of Co NWs. Increasing the duration of off-time between pulses during the electrodeposition of Co NWs made it possible to increase the amount of Cu content, so that Co-rich CoCu NWs were obtained. The parallel coercivity and squareness values increased up to 1500 Oe and 0.8 for 30 nm diameter Co94Cu6 NWs, starting from 500 Oe and 0.3 for pure Co NWs. On the other hand, although there was a substantial difference between the crystalline characteristics of 75 nm diameter pure Co and CoCu NWs, no considerable change in their magnetic properties was observed using hysteresis loop measurements. In this respect, the first-order reversal curve (FORC) analysis revealed strong inter-wire magnetostatic interactions for the CoCu NWs. Moreover, we studied the effect of thermal annealing, which resulted in an increase in the coercivity of CoCu NWs with different diameters up to 15%. As a result, the addition of small amount of Cu provides an alternative approach to tailoring the magnetic properties of Co NWs.

  12. Anisotropic thermal property of magnetically oriented carbon nanotube polymer composites

    NASA Astrophysics Data System (ADS)

    Li, Bin; Dong, Shuai; Wang, Caiping; Wang, Xiaojie; Fang, Jun

    2016-04-01

    This paper proposes a method for preparing multi-walled carbon nanotubea/polydimethylsiloxane (MWCNTs/PDMS) composites with enhanced thermal properties by using a high magnetic field (up to 10T). The MWCNT are oriented magnetically inside a silicone by in-situ polymerization method. The anisotropic structure would be expected to produce directional thermal conductivity. This study will provide a new approach to the development of anisotropic thermal-conductive polymer composites. Systematic studies with the preparation of silicone/graphene composites corresponding to their thermal and mechanical properties are carried out under various conditions: intensity of magnetic field, time, temperature, fillings. The effect of MWCNT/graphene content and preparation procedures on thermal conductivity of composites is investigated. Dynamic mechanical analysis (DMA) is used to reveal the mechanical properties of the composites in terms of the filling contents and magnetic field strength. The scanning electron microscope (SEM) is used to observe the micro-structure of the MWCNT composites. The alignment of MWCNTs in PDMS matrix is also studied by Raman spectroscopy. The thermal conductivity measurements show that the magnetically aligned CNT-composites feature high anisotropy in thermal conductivity.

  13. Magnetic properties of pulsed laser deposition-fabricated isotropic Fe-Pt film magnets

    SciTech Connect

    Nakano, M.; Oniki, W.; Yanai, T.; Fukunaga, H.

    2011-04-01

    A high-speed pulsed laser deposition method with the deposition rate of several tens of microns per 1 h enabled us to obtain isotropic Fe-Pt thick film magnets. Increase in the laser power enabled us to obtain as-deposited films with L1{sub 0} ordered phase due to the heat radiation from a target, which means that a substrate heating system and a post-annealing process are not required to achieve hard magnetic properties in the process. Use of an Fe-rich target enhanced the magnetic properties, and as a result (BH){sub max} value exceeded 100 kJ/m{sup 3} in an isotropic Fe-Pt film fabricated at the power of 3 W, which was comparable to those of isotropic Fe-Pt thick film magnets prepared by a sputtering method.

  14. Comparison of confinement in resistive-shell reversed-field pinch devices with two different magnetic shell penetration times

    NASA Astrophysics Data System (ADS)

    Gravestijn, R. M.; Drake, J. R.; Hedqvist, A.; Rachlew, E.

    2004-01-01

    A loop voltage is required to sustain the reversed-field pinch (RFP) equilibrium. The configuration is characterized by redistribution of magnetic helicity but with the condition that the total helicity is maintained constant. The magnetic field shell penetration time, tgrs, has a critical role in the stability and performance of the RFP. Confinement in the EXTRAP device has been studied with two values of tgrs, first (EXTRAP-T2) with tgrs of the order of the typical relaxation cycle timescale and then (EXTRAP-T2R) with tgrs much longer than the relaxation cycle timescale, but still much shorter than the pulse length. Plasma parameters show significant improvements in confinement in EXTRAP-T2R. The typical loop voltage required to sustain comparable electron poloidal beta values is a factor of 3 lower in the EXTRAP-T2R device. The improvement is attributed to reduced magnetic turbulence.

  15. High-power-density approaches to magnetic fusion energy: Problems and promise of compact Reversed-Field Pinch Reactors (CRFPR)

    NASA Astrophysics Data System (ADS)

    Hagenson, R. L.; Krakowski, R. A.; Dreicer, H.

    If the cost assumptions upon which the positive assessment of conventional large superconducting fusion reactors are based proves optimistic, approaches that promise considerably increased system power density and reduced mass utilization are required. These more compact reactor embodiments generally must operate with reduced shield thickness and resistive magnets. Because of the unique magnetic topology associated with the Reversed Field Pinch (RFP), the compact reactor embodiment of this approach is particularly attractive from the view point of low field resistive coils operating with Ohmic losses that are small relative to the fusion power. The RFP, one example of a high power density (HPD) approach to magnetic fusion energy. A comprehensive system model is described and applied to select a unique, cost optimized design point that is used for a subsequent conceptual engineering design of the Compact RFP Reactor.

  16. Effects of Static Magnetic Fields on the Visual Cortex: reversible Visual Deficits and Reduction of Neuronal Activity.

    PubMed

    Aguila, Jordi; Cudeiro, Javier; Rivadulla, Casto

    2016-02-01

    Noninvasive brain stimulation techniques have been successfully used to modulate brain activity, have become a highly useful tool in basic and clinical research and, recently, have attracted increased attention due to their putative use as a method for neuro-enhancement. In this scenario, transcranial static magnetic stimulation (SMS) of moderate strength might represent an affordable, simple, and complementary method to other procedures, such as Transcranial Magnetic Stimulation or direct current stimulation, but its mechanisms and effects are not thoroughly understood. In this study, we show that static magnetic fields applied to visual cortex of awake primates cause reversible deficits in a visual detection task. Complementary experiments in anesthetized cats show that the visual deficits are a consequence of a strong reduction in neural activity. These results demonstrate that SMS is able to effectively modulate neuronal activity and could be considered to be a tool to be used for different purposes ranging from experimental studies to clinical applications.

  17. Damping of Energetic-Particle-Driven Alfven Eigenmodes in Different Magnetic Equilibria in the MST Reversed-Field Pinch

    NASA Astrophysics Data System (ADS)

    Sears, Stephanie; Anderson, Jay; Capecchi, William; Bonofiglo, Phillip; Kim, Jungha

    2015-11-01

    Alfven wave dissipation is an important mechanism behind anomalous ion heating, both in astrophysical and reversed-field pinch (RFP) plasma systems. Additionally, the damping rate has implications for the stability of energetic particle driven modes (EPMs) and their associated nonlinear dynamics and fast ion transport, which are crucial topics for any burning plasma reactor. With a 1 MW neutral beam injector on the MST RFP, a controlled set of EPMs and Alfvenic eigenmodes can be driven in this never-before-probed region of strong magnetic shear and weak externally applied magnetic field. The decay time of the average of 100s of reproducible bursts is computed for different equilibrium profiles. In this work, we report initial measurements of Alfvenic damping rates with varied RFP equilibria (including magnetic shear and flow shear) and the effects on fast ion transport. This research is supported by DOE and NSF.

  18. Design and synthesis of nonionic copolypeptide hydrogels with reversible thermoresponsive and tunable physical properties.

    PubMed

    Zhang, Shanshan; Alvarez, Daniel J; Sofroniew, Michael V; Deming, Timothy J

    2015-04-13

    Polypeptide-based formulations that undergo liquid to hydrogel transitions upon change in temperature have become desirable targets since they can be mixed with cells or injected into tissues as liquids, and subsequently transform into rigid scaffolds or depots. Such materials have been challenging to prepare using synthetic polypeptides, especially when reversible gelation and tunable physical properties are desired. Here, we designed and prepared new nonionic diblock copolypeptide hydrogels (DCH) containing hydrophilic poly(γ-[2-(2-methoxyethoxy)ethyl]-rac-glutamate) and hydrophobic poly(l-leucine) segments, named DCHEO, and also further incorporated copolypeptide domains into DCHEO to yield unprecedented thermoresponsive DCH, named DCHT. Although previous attempts to prepare nonionic hydrogels composed solely of synthetic polypeptides have been unsuccessful, our designs yielded materials with highly reversible thermal transitions and tunable properties. Nonionic, thermoresponsive DCHT were found to support the viability of suspended mesenchymal stem cells in vitro and were able to dissolve and provide prolonged release of both hydrophilic and hydrophobic molecules. The versatility of these materials was further demonstrated by the independent molecular tuning of DCHT liquid viscosity at room temperature and DCHT hydrogel stiffness at elevated temperature, as well as the DCHT liquid to hydrogel transition temperature itself.

  19. Analysis of magnetic probe signals including effect of cylindrical conducting wall for field-reversed configuration experiment

    SciTech Connect

    Ikeyama, Taeko; Hiroi, Masanori; Nemoto, Yuuichi; Nogi, Yasuyuki

    2008-06-15

    A confinement field is disturbed by magnetohydrodynamic (MHD) motions of a field-reversed configuration (FRC) plasma in a cylindrical conductor. The effect of the conductor should be included to obtain a spatial structure of the disturbed field with a good precision. For this purpose, a toroidal current in the plasma and an eddy current on a conducting wall are replaced by magnetic dipole and image magnetic dipole moments, respectively. Typical spatial structures of the disturbed field are calculated by using the dipole moments for such MHD motions as radial shift, internal tilt, external tilt, and n=2 mode deformation. Then, analytic formulas for estimating the shift distance, tilt angle, and deformation rate of the MHD motions from magnetic probe signals are derived. It is estimated from the calculations by using the dipole moments that the analytic formulas include an approximately 40% error. Two kinds of experiment are carried out to investigate the reliability of the calculations. First, a magnetic field produced by a circular current is measured in an aluminum pipe to confirm the replacement of the eddy current with the image magnetic dipole moments. The measured fields coincide well with the calculated values including the image magnetic dipole moments. Second, magnetic probe signals measured from the FRC plasma are substituted into the analytic formulas to obtain shift distance and deformation rate. The experimental results are compared to the MHD motions measured by using a radiation from the plasma. If the error included in the analytic formulas and the difference between the magnetic and optical structures in the plasma are considered, the results of the radiation measurement support well those of the magnetic analysis.

  20. Evidence for the Reversal of Magnetic Field Polarity in Coronal Streamers

    NASA Technical Reports Server (NTRS)

    Woo, Richard

    1996-01-01

    Faraday rotation observations are unique amongst radio occultation measurements in that they respond to magnetic field in addition to electron density, making it possible to probe the coronal magnetic field.