Continuous 1052, 1064 nm dual-wavelength Nd:YAG laser

NASA Astrophysics Data System (ADS)

Wang, Xiaozhong; Yuan, Haiyang; Wang, Mingshan; Huang, Wencai

2016-10-01

Dual-wavelength lasers are usually obtained through balancing the net gain of the two oscillating lines. Competition between transitions 1052 nm, 1061 nm and 1064 nm is utilized to realize a continuous wave 1052 and 1064 nm dual-wavelength Nd:YAG laser firstly in this paper. A specially designed Fabry-Perot band-pass filter is exploited as output coupler to control the thresholds of the oscillating wavelengths. The maximum power of the dual-wavelength laser is 1.6 W and the slope efficiency is about 10%. The power instability of the output dual-wavelength laser is smaller than ±4% in half an hour. The mechanism presented in this paper may provide a new way to obtain dual-wavelength lasers.

Demonstration of a neonlike argon soft-x-ray laser with a picosecond-laser-irradiated gas puff target.

PubMed

Fiedorowicz, H; Bartnik, A; Dunn, J; Smith, R F; Hunter, J; Nilsen, J; Osterheld, A L; Shlyaptsev, V N

2001-09-15

We demonstrate a neonlike argon-ion x-ray laser, using a short-pulse laser-irradiated gas puff target. The gas puff target was formed by pulsed injection of gas from a high-pressure solenoid valve through a nozzle in the form of a narrow slit and irradiated with a combination of long, 600-ps and short, 6-ps high-power laser pulses with a total of 10 J of energy in a traveling-wave excitation scheme. Lasing was observed on the 3p (1)S(0)?3s (1)P(1) transition at 46.9 nm and the 3d (1)P(1)?3p (1)P(1) transition at 45.1 nm. A gain of 11 cm(-1) was measured on these transitions for targets up to 0.9 cm long.

Kinetic model of stimulated emission created by resonance pumping of aluminum laser-induced plasma

NASA Astrophysics Data System (ADS)

Gornushkin, I. B.; Kazakov, A. Ya.

2017-06-01

Stimulated emission observed experimentally in an aluminum laser induced plasma is modeled via a kinetic approach. The simulated emission at several cascade transitions is created by a pump laser guided through the plasma at several microseconds after its creation and tuned in resonance with the strong 3s23p-3s24s transition at 266 nm. A two-dimensional space-time collisional radiative plasma model explains the creation of the population inversion and lasing at wavelengths of 2100 n m and 396.1 nm. The population inversion for lasing at 2100 n m is created by depopulation of the ground 3s23p state and population of the 3s25s state via the absorption of the resonant radiation at 266 nm. The population inversion for lasing at 396.1 nm occurs during the laser pulse via the decay of the population of the pumped 3s25s state to the excited 3s24s state via cascade transitions driven optically and by collisions. In particular, efficient are the mixing transitions between neighboring states separated by small gaps on the order of k T at plasma temperatures of 5000-10 000 K. The model predicts that the population inversion and corresponding gain may reach high values even at very moderate pump energy of several μJ per pulse. The efficiency of lasing at 2100 n m and 396.1 nm is estimated to be ˜3% and 0.05%, correspondingly with respect to the pump laser intensity. The gain for lasing at 396.1 nm can reach as high as ˜40 cm-1. The polarization effect that the pump radiation at 266 nm imposes on the stimulated emission at 396.1 nm is discussed. The calculated results are favorably compared to experimental data.

Temperature dependence of quasi-three level laser transition for long pulse Nd:YAG laser

NASA Astrophysics Data System (ADS)

Bidin, Noriah; Pourmand, Seyed Ebrahim; Sidi Ahmad, Muhamad Fakaruddin; Khrisnan, Ganesan; Mohd Taib, Nur Athirah; Nadia Adnan, Nurul; Bakhtiar, Hazri

2013-02-01

The influence of temperature and pumping energy on stimulated emission cross section and the laser output of quasi-three level laser transition are reported. Flashlamp is used to pump Nd:YAG laser rod. Distilled water is mixed with ethylene glycol to vary the temperature of the cooling system between -30 and 60 °C. The capacitor voltage of flashlamp driver is verified to manipulate the input energy within the range of 10-70 J. The line of interest in quasi-three level laser comprised of 938.5 and 946 nm. The stimulated emission cross section of both lines is found to be inversely proportional to the temperature but directly proportional to the input energy. This is attributed from thermal broadening effect. The changes of stimulated emission cross section and the output laser with respect to the temperature and input energy on line 946 nm are realized to be more dominant in comparison to 938.5 nm.

Coupled optical resonance laser locking.

PubMed

Burd, S C; du Toit, P J W; Uys, H

2014-10-20

We have demonstrated simultaneous laser frequency stabilization of a UV and IR laser, to coupled transitions of ions in the same spectroscopic sample, by detecting only the absorption of the UV laser. Separate signals for locking the different lasers are obtained by modulating each laser at a different frequency and using lock-in detection of a single photodiode signal. Experimentally, we simultaneously lock a 369 nm and a 935 nm laser to the (2)S(1/2) → (2)(P(1/2) and (2)D(3/2) → (3)D([3/2]1/2) transitions, respectively, of Yb(+) ions generated in a hollow cathode discharge lamp. Stabilized lasers at these frequencies are required for cooling and trapping Yb(+) ions, used in quantum information and in high precision metrology experiments. This technique should be readily applicable to other ion and neutral atom systems requiring multiple stabilized lasers.

All-solid-state continuous-wave frequency doubling Nd:LuVO4/LBO laser with 2.17 W output power at 543 nm

NASA Astrophysics Data System (ADS)

Li, B.; Zhao, L.; Zhang, Y. B.; Zheng, Q.; Zhao, Y.; Yao, Y.

2013-03-01

Efficient and compact green-yellow laser output at 543 nm is generated by intracavity frequency doubling of a CW diode-pumped Nd:LuVO4 laser at 1086 nm under the condition of suppressing the higher gain transition near 1064 nm. With 16 W of diode pump power and the frequency-doubling crystal LBO, as high as 2.17 W of CW output power at 543 nm is achieved, corresponding to an optical-to-optical conversion efficiency of 13.6% and the output power stability over 8 hours is better than 2.86%. To the best of our knowledge, this is the highest watt-level laser at 543 nm generated by intracavity frequency doubling of a diode pumped Nd:LuVO4 laser at 1086 nm.

Discrete multi-wavelength tuning of a continuous wave diode-pumped Nd:GdVO4 laser

NASA Astrophysics Data System (ADS)

Nadimi, Mohammad; Waritanant, Tanant; Major, Arkady

2018-05-01

Discrete multi-wavelength operation of a diode-pumped Nd:GdVO4 laser at four different wavelengths was demonstrated using a single birefringent filter plate. The laser achieved maximum output powers of 5.92 W, 5.66 W, 5.56 W and 3.98 W at 1063.2 nm, 1070.8 nm, 1082.5 nm and 1086.2 nm wavelengths, respectively. To the best of our knowledge, apart from achieving the maximum output powers at ~1071 nm and ~1086 nm and best efficiencies at ~1071 nm, ~1083 nm and ~1086 nm wavelengths for a Nd:GdVO4 laser, this is also the largest number of wavelengths from the 4F3/2  →  4I11/2 transition that was ever obtained in a controlled manner from a single laser setup based on any of the Nd-doped laser crystals.

Blue-green upconversion laser

DOEpatents

Nguyen, D.C.; Faulkner, G.E.

1990-08-14

A blue-green laser (450--550 nm) uses a host crystal doped with Tm[sup 3+]. The Tm[sup 3+] is excited through upconversion by a red pumping laser and an IR pumping laser to a state which transitions to a relatively lower energy level through emissions in the blue-green band, e.g., 450.20 nm at 75 K. The exciting laser may be tunable dye lasers or may be solid-state semiconductor laser, e.g., GaAlAs and InGaAlP. 3 figs.

Blue-green upconversion laser

DOEpatents

Nguyen, Dinh C.; Faulkner, George E.

1990-01-01

A blue-green laser (450-550 nm) uses a host crystal doped with Tm.sup.3+. The Tm.sup.+ is excited through upconversion by a red pumping laser and an IR pumping laser to a state which transitions to a relatively lower energy level through emissions in the blue-green band, e.g., 450.20 nm at 75 K. The exciting laser may be tunable dye lasers or may be solid-state semiconductor laser, e.g., GaAlAs and InGaAlP.

Standoff analysis of laser-produced plasmas using laser-induced fluorescence

DOE Office of Scientific and Technical Information (OSTI.GOV)

Harilal, S. S.; Brumfield, B. E.; Phillips, M. C.

We report the use of laser-induced fluorescence (LIF) of laser ablation plumes for standoff applications. The standoff analysis of Al species, as major and minor species in samples, is performed in a nanosecond laser-produced plasma created at a distance ~10 m. The LIF analysis is performed by resonantly exciting an Al transition at 394.4 nm using a continuous wave (cw) tunable laser and by collecting the direct-line fluorescence signal at 396.15 nm. The spectral resolution of LIF is obtained by scanning the cw tunable LIF laser across the selected Al transition. Our results highlight that LIF provides enhanced signal intensity,more » emission persistence, and spectral resolution when compared to thermally-excited emission, and these are crucial considerations for using laser-produced plasma for standoff isotopic analysis.« less

Laser diode and pumped Cr:Yag passively Q-switched yellow-green laser at 543 nm

NASA Astrophysics Data System (ADS)

Yao, Y.; Ling, Zhao; Li, B.; Qu, D. P.; Zhou, K.; Zhang, Y. B.; Zhao, Y.; Zheng, Q.

2013-03-01

Efficient and compact yellow green pulsed laser output at 543 nm is generated by frequency doubling of a passively Q-switched end diode-pumped Nd:YVO4 laser at 1086 nm under the condition of sup-pressing the higher gain transition near 1064 nm. With 15 W of diode pump power and the frequency doubling crystal LBO, as high as 1.58 W output power at 543 nm is achieved. The optical to optical conversion efficiency from the corresponding Q-switched fundamental output to the yellow green output is 49%. The peak power of the Q-switched yellow green pulse laser is up to 30 kW with 5 ns pulse duration. The output power stability over 8 hours is better than 2.56% at the maximum output power. To the best of our knowledge, this is the highest watt-level laser at 543 nm generated by frequency doubling of a passively Q-switched end diode pumped Nd:YVO4 laser at 1086 nm.

Analysis of soft x-ray emission spectra of laser-produced dysprosium, erbium and thulium plasmas

NASA Astrophysics Data System (ADS)

Sheil, John; Dunne, Padraig; Higashiguchi, Takeshi; Kos, Domagoj; Long, Elaine; Miyazaki, Takanori; O'Reilly, Fergal; O'Sullivan, Gerard; Sheridan, Paul; Suzuki, Chihiro; Sokell, Emma; White, Elgiva; Kilbane, Deirdre

2017-03-01

Soft x-ray emission spectra of dysprosium, erbium and thulium ions created in laser-produced plasmas were recorded with a flat-field grazing-incidence spectrometer in the 2.5-8 nm spectral range. The ions were produced using an Nd:YAG laser of 7 ns pulse duration and the spectra were recorded at various power densities. The experimental spectra were interpreted with the aid of the Cowan suite of atomic structure codes and the flexible atomic code. At wavelengths above 5.5 nm the spectra are dominated by overlapping n = 4 - n = 4 unresolved transition arrays from adjacent ion stages. Below 6 nm, n = 4 - n = 5 transitions also give rise to a series of interesting overlapping spectral features.

Control system high-precision laser to obtain the ensemble of ultracold ions Th3+

NASA Astrophysics Data System (ADS)

Florentsev, V. V.; Zhdamirov, V. Yu; Rodko, I. I.; Borodulya, N. A.; Biryukov, A. P.

2018-01-01

One of key problems of nuclear standard frequency development is preparation assembly of ultracold thorium ions in Pauli trap. In this case semiconductive frequency-stabilized lasers with external resonator on frequencies 690 nm, 984 nm, and 1088 nm are used for excitation of corresponding electronic dipole and quadrupole cooling transitions for Th3+ ions. In the paper the results of development and creation of unified laser module, which is able to be used as base for full-featured system designed for laser cooling of Th3+ ions, are presented. The module is able to fine-tune necessary wavelength with accuracy ±5 nm.

Development of Two-Photon Pump Polarization Spectroscopy Probe Technique Tpp-Psp for Measurements of Atomic Hydrogen .

NASA Astrophysics Data System (ADS)

Satija, Aman; Lucht, Robert P.

2015-06-01

Atomic hydrogen (H) is a key radical in combustion and plasmas. Accurate knowledge of its concentration can be used to better understand transient phenomenon such as ignition and extinction in combustion environments. Laser induced polarization spectroscopy is a spatially resolved absorption technique which we have adapted for quantitative measurements of H atom. This adaptation is called two-photon pump, polarization spectroscopy probe technique (TPP-PSP) and it has been implemented using two different laser excitation schemes. The first scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-3P levels using a circularly polarized 656-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 656 nm. As a result, the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. The laser beams were created by optical parametric generation followed by multiple pulse dye amplification stages. This resulted in narrow linewidth beams which could be scanned in frequency domain and varied in energy. This allowed us to systematically investigate saturation and Stark effect in 2S-3P transitions with the goal of developing a quantitative H atom measurement technique. The second scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-4P transitions using a circularly polarized 486-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 486 nm. As a result the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. A dye laser was pumped by third harmonic of a Nd:YAG laser to create a laser beam at 486 nm. The 486-nm beam was frequency doubled to a 243-nm beam. Use of the second scheme simplifies the TPP-PSP technique making it more convenient for diagnostics in practical systems.

Two-Photon/Laser-Induced Fluorescence (TP/LIF) sensor

NASA Technical Reports Server (NTRS)

Bradshaw, John D.

1994-01-01

The Two-Photon/Laser-Induced Fluorescence (TP/LIF) technique is based on the stepwise excitation of the OH transitions, X(exp 2)II, v(exp '') = 0 yields X(exp 2)II, v(exp '') = 1 (lambda = 2.9 microns) and X(exp 2)II v(exp '') = 1 yields A(exp2)Sigma, v' = 0 (lambda = 345 nm) with background free fluorescence monitoring of the A(exp 2)Sigma, v' = 0 yields X(exp 2)II, v(exp '') = 0 transition near 309 nm. This technique has awaited the advent of a suitable mid-infrared (2.9 microns) laser source. Turnable mid-IR lasers now exist that are capable of meeting the specifications required of a high sensitivity TP/LIF OH sensor.

Laser optogalvanic wavelength calibration with a commercial hollow cathode iron - neon discharge lamp

NASA Technical Reports Server (NTRS)

Zhu, Xinming; Nur, Abdullahi H.; Misra, Prabhakar

1994-01-01

351 optogalvanic transitions have been observed in the 337 - 598 nm wavelength region using an iron - neon hollow cathode discharge lamp and a pulsed tunable dye laser. 223 of these have been identified as transitions associated with neon energy levels. These optogalvanic transitions have allowed, in conjunction with interference fringes recorded concomitantly with an etalon, the calibration of the dye laser wavelength with 0.3/cm accuracy.

Influence of laser wavelength on two-dimensional carbon nanosheet formation from laser-induced exfoliation of naphthalene

NASA Astrophysics Data System (ADS)

Qian, Min; Niu, Yue Ping; Gong, Shang Qing

2018-01-01

Pulsed Nd:YAG (532 nm) and Excimer (248 nm) lasers were employed to produce freestanding, two-dimensional (2D), carbon nanosheets (CNSs) from naphthalene, through laser-induced exfoliation. The polymer-to-carbon transition was investigated in terms of laser wavelengths, fluences, as well as target preparations. Continuous and porous CNSs of several nanometers in thickness and micrometers in size were obtained from 532 and 248 nm pulsed laser exfoliation of spin-coated naphthalene films, respectively. The porous morphology is ascribed to the photon-induced dissociation of chemical bonds dominated in 248 nm laser interaction with ablated naphthalene. With the increase of laser fluences from 1 to 5 J cm-2, amorphous carbon and ultrathin CNS structures were obtained in sequence. This work revealed a general mechanism of producing 2D structured carbon materials from pulsed laser exfoliation.

Scalable waveguide design for three-level operation in Neodymium doped fiber laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pax, Paul H.; Khitrov, Victor V.; Drachenberg, Derrek R.

We have constructed a double clad neodymium doped fiber laser operating on the three-level 4F 3/2 → 4I 9/2 transition. The laser has produced 11.5 W at 925 nm with 55% slope efficiency when pumped at 808 nm, comparable to the best previous results for a double-clad fiber configuration on this transition. Higher power pumping with both 808 nm and 880 nm sources resulted in an output of 27 W, albeit at lower slope efficiency. In both cases, output power was limited by available pump, indicating the potential for further power scaling. To suppress the stronger four-level 4F 3/2 →more » 4I 11/2 transition we developed a waveguide that provides spectral filtering distributed along the length of the fiber, based on an all-solid micro-structured optical fiber design, with resonant inclusions creating a leakage path to the cladding. Furthermore, the waveguide supports large mode areas and provides strong suppression at selectable wavelength bands, thus easing the restrictions on core and cladding sizes that limited power scaling of previous approaches.« less

Scalable waveguide design for three-level operation in Neodymium doped fiber laser

DOE PAGES

Pax, Paul H.; Khitrov, Victor V.; Drachenberg, Derrek R.; ...

2016-12-12

We have constructed a double clad neodymium doped fiber laser operating on the three-level 4F 3/2 → 4I 9/2 transition. The laser has produced 11.5 W at 925 nm with 55% slope efficiency when pumped at 808 nm, comparable to the best previous results for a double-clad fiber configuration on this transition. Higher power pumping with both 808 nm and 880 nm sources resulted in an output of 27 W, albeit at lower slope efficiency. In both cases, output power was limited by available pump, indicating the potential for further power scaling. To suppress the stronger four-level 4F 3/2 →more » 4I 11/2 transition we developed a waveguide that provides spectral filtering distributed along the length of the fiber, based on an all-solid micro-structured optical fiber design, with resonant inclusions creating a leakage path to the cladding. Furthermore, the waveguide supports large mode areas and provides strong suppression at selectable wavelength bands, thus easing the restrictions on core and cladding sizes that limited power scaling of previous approaches.« less

A frequency-stabilized light source at 399 nm using an Yb hollow-cathode lamp

NASA Astrophysics Data System (ADS)

Tanabe, Takehiko; Akamatsu, Daisuke; Inaba, Hajime; Okubo, Sho; Kobayashi, Takumi; Yasuda, Masami; Hosaka, Kazumoto; Hong, Feng-Lei

2018-06-01

We demonstrate a diode laser system operating at 399 nm that is stabilized to the 6s2 1S0–6s6p 1P1 electric dipole transition in ytterbium (Yb) atoms in a hollow-cathode lamp. The frequency stability of the laser reached 1.1 × 10‑11 at an averaging time of τ = 1 s. We performed an absolute frequency measurement using an optical frequency comb and determined that the absolute frequency of the laser stabilized to the 1S0–1P1 transition in 174Yb was 751 526 522.26(9) MHz. We also investigated several systematic frequency shifts while changing some of the light source parameters and measured several isotope shifts. The measured laser frequency will provide useful information regarding the practical use of the frequency-stabilized light source at 399 nm.

Diode-pumped cw Nd:YAG three-level laser at 869 nm.

PubMed

Lü, Yanfei; Xia, Jing; Cheng, Weibo; Chen, Jifeng; Ning, Guobin; Liang, Zuoliang

2010-11-01

We report for the first time (to our knowledge) a diode-pumped Nd:YAG laser emitting at 869 nm based on the (4)F(3/2)-(4)I(9/2) transition, generally used for a 946 nm emission. Power of 453 mW at 869 nm has been achieved in cw operation with a fiber-coupled laser diode emitting 35.4 W at 809 nm. Intracavity second-harmonic generation in the cw mode has also been demonstrated with power of 118 mW at 435 nm by using a BiB(3)O(6) nonlinear crystal. In our experiment, we used a LiNbO(3) crystal lens to complement the thermal lens of the laser rod, and we obtained good beam quality and high output power stability.

Disordered Nd:LuYSiO5 crystal lasers operating on the 4F3/2 → 4I11/2 and 4F3/2 → 4I13/2 transitions

NASA Astrophysics Data System (ADS)

Guan, Xiaofeng; Zhou, Zhiyong; Huang, Xiaoxu; Xu, Bin; Xu, Huiying; Cai, Zhiping; Xu, Xiaodong; Xu, Jun

2017-11-01

We report on diode-pumped disordered Nd:LuYSiO5 (Nd:LYSO) crystal lasers operating on the 4F3/2 → 4I11/2 and 4F3/2 → 4I 13/2 transitions. Simultaneous laser operation at 1074 and 1078 nm is achieved with maximum output power of 4.46 W and slope efficiency of 39.6%. Single wavelength laser at 1358 nm with maximum output power of 1.15 W and slope efficiency of 11.8% is also obtained. Moreover, four single-wavelength lasers at 1058, 1107, 1330 and 1386 nm with relatively low gains are achieved with maximum output powers of 2.72, 1.22, 0.52 and 0.42 W, respectively, for the first time to our knowledge. Lasing at non-traditional emission lines was obtained by using output couplers with dielectric coatings for specific wavelength ranges.

Carbon dioxide laser polishing of fused silica surfaces for increased laser-damage resistance at 1064 nm.

PubMed

Temple, P A; Lowdermilk, W H; Milam, D

1982-09-15

Mechanically polished fused silica surfaces were heated with continuous-wave CO(2) laser radiation. Laser-damage thresholds of the surfaces were measured with 1064-nm 9-nsec pulses focused to small spots and with large-spot, 1064-nm, 1-nsec irradiation. A sharp transition from laser-damage-prone to highly laser-damage-resistant took place over a small range in CO(2) laser power. The transition to high damage resistance occurred at a silica surface temperature where material softening began to take place as evidenced by the onset of residual strain in the CO(2) laser-processed part. The small-spot damage measurements show that some CO(2) laser-treated surfaces have a local damage threshold as high as the bulk damage threshold of SiO(2). On some CO(2) laser-treated surfaces, large-spot damage thresholds were increased by a factor of 3-4 over thresholds of the original mechanically polished surface. These treated parts show no obvious change in surface appearance as seen in bright-field, Nomarski, or total internal reflection microscopy. They also show little change in transmissive figure. Further, antireflection films deposited on CO(2) laser-treated surfaces have thresholds greater than the thresholds of antireflection films on mechanically polished surfaces.

Dual-axis vapor cell for simultaneous laser frequency stabilization on disparate optical transitions

NASA Astrophysics Data System (ADS)

Jayakumar, Anupriya; Plotkin-Swing, Benjamin; Jamison, Alan O.; Gupta, Subhadeep

2015-07-01

We have developed a dual-axis ytterbium (Yb) vapor cell and used it to simultaneously address the two laser cooling transitions in Yb at wavelengths 399 nm and 556 nm, featuring the disparate linewidths of 2π × 29 MHz and 2π × 182 KHz, respectively. By utilizing different optical paths for the two wavelengths, we simultaneously obtain comparable optical densities suitable for saturated absorption spectroscopy for both the transitions and keep both the lasers frequency stabilized over several hours. We demonstrate that by appropriate control of the cell temperature profile, two atomic transitions differing in relative strength across a large range of over three orders of magnitude can be simultaneously addressed, making the device adaptable to a variety of spectroscopic needs. We also show that our observations can be understood with a simple theoretical model of the Yb vapor.

Experimental investigation of a pulsed Rb-Ar excimer-pumped alkali laser

NASA Astrophysics Data System (ADS)

Cheng, Hongling; Wang, Zhimin; Zhang, Fengfeng; Wang, Mingqiang; Tian, Zhaoshuo; Peng, Qinjun; Cui, Dafu; Xu, Zuyan

2017-03-01

We present experimental results of an exciplex-pumped alkali laser (XPAL) at 780 nm based on the 52P3/2 → 52S1/2 transition of the Rb atom in mixtures of Rb vapor and Ar. A laboratory-built Ti:sapphire laser with a pulse repetition rate of 3 kHz and a pulse width of 100 ns is used as the pump source. The maximum laser pulse energy of 0.26 µJ at 780 nm is obtained under an absorbed pump pulse energy of 42 µJ at 755 nm in mixtures of Rb vapor and Ar at a temperature of 423 K, corresponding to an optical conversion efficiency of 0.62%. Further experiments show that the output laser at 780 nm can always be detected for pump wavelengths ranging from 754 to 759 nm, indicating that Rb-Ar mixtures can be effectively pumped by commercial laser diodes (LDs) with a bandwidth of 5 nm.

Femtosecond-pulse-driven electron-excited extreme-ultraviolet lasers in Be-like ions.

PubMed

Hooker, S M; Harris, S E

1995-10-01

A suggestion for the generation of extreme-ultraviolet (XUV) laser radiation based on tunneling ionization and subsequent electron excitation of Deltan not equal 0 transitions is described. The favorable scaling of the required intensity of the pump laser with the output XUV wavelength is compared with that exhibited by XUV lasers ased on Deltan = 0 transitions. Calculations for Be-like Ne predict signif icant gain at 14.1 nm.

All-solid-state cw frequency-doubling Nd:YLiF4/LBO blue laser with 4.33 W output power at 454 nm under in-band diode pumping at 880 nm.

PubMed

Lü, Yanfei; Zhang, Xihe; Cheng, Weibo; Xia, Jing

2010-07-20

We generated efficient blue laser output at 454 nm by intracavity frequency doubling of a continuous-wave (cw) diode-pumped Nd:YLiF(4) (Nd:YLF) laser at 908 nm based on the (4)F(3/2)-(4)I(9/2) transition. With 32.8 W of incident pump power at 880 nm and the frequency-doubling crystal LiB(3)O(5), a level as high as 4.33 W of cw output power at 454 nm is achieved, corresponding to an optical conversion efficiency of 13.2% with respect to the incident pump power. To the best of our knowledge, this is the first blue laser at 454 nm generated by intracavity frequency doubling of a diode-pumped Nd:YLF.

Enhancement of 800 nm upconversion emission in a thulium doped tellurite microstructured fiber pumped by a 1560 nm femtosecond fiber laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jia, Zhixu; Zheng, Kezhi; State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, Changchun 130012

We report enhanced upconversion (UC) fluorescence in Tm{sup 3+} doped tellurite microstructured fibers (TDTMFs) fabricated by using a rod-in-tube method. Under the pumping of a 1560 nm femtosecond fiber laser, ultrabroadband supercontinuum light expanding from ∼1050 to ∼2700 nm was generated in a 4 cm long TDTMF. Simultaneously, intense 800 nm UC emission from the {sup 3}H{sub 4} → {sup 3}H{sub 6} transition of Tm{sup 3+} was observed in the same TDTMF. Compared to that pumped by a 1560 nm continuous wave fiber laser, the UC emission intensity was enhanced by ∼4.1 times. The enhancement was due to the spectral broadening in the TDTMF under themore » pumping of the 1560 nm femtosecond fiber laser.« less

Laser characteristics at 1535 nm and thermal effects of an Er:Yb phosphate glass microchip pumped by Ti:sapphire laser

NASA Astrophysics Data System (ADS)

Cai, Zhiping; Chardon, Alain; Xu, Huiying; Féron, Patrice; Michel Stéphan, Guy

2002-03-01

An Er:Yb codoped phosphate glass microchip laser has been studied under pumping with a Ti:sapphire laser ranging from 945 to 990 nm. The characteristics (threshold, slope efficiency) are first described for an optimized laser. The gain spectrum is calculated for the transition 4I13/2→ 4I15/2 around 1535 nm from fundamental spectroscopic data and from experimental results. Red-shift effect on the frequency of a single mode is experimentally observed when the pump power is increased, originating from thermal effects. Temperature inside the microchip cavity and thermal expansion coefficient were determined by employing the intensity ratio of two green upconversion emission line centered at 530 and 554 nm, respectively, which quantitatively explain this red shift.

Red laser-diode pumped 806 nm Tm3+: ZBLAN fibre laser

NASA Astrophysics Data System (ADS)

Juárez-Hernández, M.; Mejía, E. B.

2017-06-01

A Tm3+-doped fluorozirconate (ZBLAN) fibre laser operating CW at 806 nm when diode-pumped at 687 nm is described for the first time. This device is based on the 3F4  →  3H6 transition, and is suitable for first telecom window and sensing applications. A slope efficiency of 50.3% and low threshold pump-power of 11.6 mW were obtained. Maximum output power of 15 mW for 40 mW coupled pump was achieved.

Effects of 946-nm thermal shift and broadening on Nd3+:YAG laser performance

NASA Astrophysics Data System (ADS)

Seyed Ebrahim, Pourmand; Ghasem, Rezaei

2015-12-01

Spectroscopic properties of flashlamp pumped Nd3+:YAG laser are studied as a function of temperature in a range from -30 °C to 60 °C. The spectral width and shift of quasi three-level 946.0-nm inter-Stark emission within the respective intermanifold transitions of 4F3/2 → 4I9/2 are investigated. The 946.0-nm line shifts toward the shorter wavelength and broadens. In addition, the threshold power and slope efficiency of the 946.0-nm laser line are quantified with temperature. The lower the temperature, the lower the threshold power is and the higher the slope efficiency of the 946.0-nm laser line is, thus the higher the laser output is. This phenomenon is attributed to the ion-phonon interaction and the thermal population in the ground state. Project supported by Estahban Branch, Islamic Azad University.

Simultaneous triple 914 nm, 1084 nm, and 1086 nm operation of a diode-pumped Nd:YVO4 laser

NASA Astrophysics Data System (ADS)

Lü, Yanfei; Xia, Jing; Liu, Huilong; Pu, Xiaoyun

2014-10-01

We report a diode-pumped continuous-wave (cw) triple-wavelength Nd:YVO4 laser operating at 914, 1084, and 1086 nm. A theoretical analysis has been introduced to determine the threshold conditions for simultaneous triple-wavelength laser. Using a T-shaped cavity, we realized an efficient triple-wavelength operation at 4F3/2→4I9/2 and 4F3/2→4I11/2 transitions for Nd:YVO4 crystal, simultaneously. At an absorbed pump power of 16 W (or 25 W of incident pump power), the maximum output power was 2.3 W, which included 914 nm, 1084 nm, and 1086 nm three wavelengths, and the optical conversion efficiency with respect to the absorbed pump power was 14.4%.

Efficient, diode-pumped Tm3+:BaY2F8 vibronic laser

NASA Astrophysics Data System (ADS)

Cornacchia, F.; Parisi, D.; Bernardini, C.; Toncelli, A.; Tonelli, M.

2004-05-01

In this work we report the spectroscopy and laser results of several Thulium doped BaY2F8 single crystals grown using the Czochralski technique. The doping concentration is between 2at.% and 18at.%. We performed room temperature laser experiments pumping the samples with a laser diode at 789 nm obtaining 61% as maximum optical-to-optical efficiency with a maximum output power of 290 mW and a minimum lasing threshold of 26 mW. The lasing wavelength changed with the dopant concentration from 1927 nm up to 2030 nm and the nature of the transition changed from purely electronic to vibronic, accordingly.

Resonance Raman scattering of β-carotene solution excited by visible laser beams into second singlet state.

PubMed

Lu, Luyao; Shi, Lingyan; Secor, Jeff; Alfano, Robert

2018-02-01

This study aimed to use self-absorption correction to determine the Raman enhancement of β-carotene. The Raman spectra of β-carotene solutions were measured using 488nm, 514nm, 532nm and 633nm laser beams, which exhibited significant resonance Raman (RR) enhancement when the laser energy approaches the electronic transition energy from S 0 to S 2 state. The Raman intensity and the actual resonance Raman gain without self-absorption from S 2 state by β-carotene were also obtained to evaluate the effect of self-absorption on RR scattering. Moreover, we observed the Raman intensity strength followed the absorption spectra. Our study found that, although 488nm and 514nm pumps seemed better for stronger RR enhancement, 532nm would be the optimum Raman pump laser with moderate RR enhancement due to reduced fluorescence and self-absorption. The 532nm excitation will be helpful for applying resonance Raman spectroscopy to investigate biological molecules in tissues. Copyright © 2017 Elsevier B.V. All rights reserved.

Low intensity 635 nm diode laser irradiation inhibits fibroblast-myofibroblast transition reducing TRPC1 channel expression/activity: New perspectives for tissue fibrosis treatment.

PubMed

Sassoli, Chiara; Chellini, Flaminia; Squecco, Roberta; Tani, Alessia; Idrizaj, Eglantina; Nosi, Daniele; Giannelli, Marco; Zecchi-Orlandini, Sandra

2016-03-01

Low-level laser therapy (LLLT) or photobiomodulation therapy is emerging as a promising new therapeutic option for fibrosis in different damaged and/or diseased organs. However, the anti-fibrotic potential of this treatment needs to be elucidated and the cellular and molecular targets of the laser clarified. Here, we investigated the effects of a low intensity 635 ± 5 nm diode laser irradiation on fibroblast-myofibroblast transition, a key event in the onset of fibrosis, and elucidated some of the underlying molecular mechanisms. NIH/3T3 fibroblasts were cultured in a low serum medium in the presence of transforming growth factor (TGF)-β1 and irradiated with a 635 ± 5 nm diode laser (continuous wave, 89 mW, 0.3 J/cm(2) ). Fibroblast-myofibroblast differentiation was assayed by morphological, biochemical, and electrophysiological approaches. Expression of matrix metalloproteinase (MMP)-2 and MMP-9 and of Tissue inhibitor of MMPs, namely TIMP-1 and TIMP-2, after laser exposure was also evaluated by confocal immunofluorescence analyses. Moreover, the effect of the diode laser on transient receptor potential canonical channel (TRPC) 1/stretch-activated channel (SAC) expression and activity and on TGF-β1/Smad3 signaling was investigated. Diode laser treatment inhibited TGF-β1-induced fibroblast-myofibroblast transition as judged by reduction of stress fibers formation, α-smooth muscle actin (sma) and type-1 collagen expression and by changes in electrophysiological properties such as resting membrane potential, cell capacitance and inwardly rectifying K(+) currents. In addition, the irradiation up-regulated the expression of MMP-2 and MMP-9 and downregulated that of TIMP-1 and TIMP-2 in TGF-β1-treated cells. This laser effect was shown to involve TRPC1/SAC channel functionality. Finally, diode laser stimulation and TRPC1 functionality negatively affected fibroblast-myofibroblast transition by interfering with TGF-β1 signaling, namely reducing the expression of Smad3, the TGF-β1 downstream signaling molecule. Low intensity irradiation with 635 ± 5 nm diode laser inhibited TGF-β1/Smad3-mediated fibroblast-myofibroblast transition and this effect involved the modulation of TRPC1 ion channels. These data contribute to support the potential anti-fibrotic effect of LLLT and may offer further informations for considering this therapy as a promising therapeutic tool for the treatment of tissue fibrosis. © 2015 Wiley Periodicals, Inc.

Simultaneous dual-wavelength lasing at 1047 and 1053 nm and wavelength tuning to 1072 nm in a diode-pumped a-cut Nd : LiYF4 laser

NASA Astrophysics Data System (ADS)

Lin, Zhi; Wang, Yi; Xu, Bin; Cheng, Yongjie; Xu, Huiying; Cai, Zhiping

2015-12-01

We report on diode-end-pumped a-cut Nd:YLF laser on F→I transition. In a free-running regime, using an output coupler with a radius of curvature of 1000 mm, we obtain dual-wavelength laser operation at both π-polarized 1047 nm and σ-polarized 1053 nm with maximum output power of about 1.25 W and the highest slope efficiency of about 50.9% at pump power of 5.77 W at room temperature, for the first time to our knowledge. Furthermore, using a 0.1-mm glass plate as a wavelength selector, a dual-wavelength laser at 1047 and 1072 nm can also be yielded with the maximum output power of 0.34 W, which has not been reported before.

Cascade generation in Al laser induced plasma

NASA Astrophysics Data System (ADS)

Nagli, Lev; Gaft, Michael; Raichlin, Yosef; Gornushkin, Igor

2018-05-01

We found cascade IR generation in Al laser induced plasma. This generation includes doublet transitions 3s 25s 2S1/2 → 3s24p 2P1/2,3/2 → 3s24s 2S1/2; corresponding to strong lines at 2110 and 2117 nm, and much weaker lines at 1312-1315 nm. The 3s25s2S 1/2 starting IR generation level is directly pumped from the 3s23p 2P3/2 ground level. The starting level for UV generation at 396.2 nm (transitions 3s24s 2S1/2 → 4p 2P3/2) is populated due to the fast collisional processes in the plasma plume. These differences led to different time and special dependences on the lasing in the IR and UV spectral range within the aluminum laser induced plasma.

Laser-induced fluorescence detection strategies for sodium atoms and compounds in high-pressure combustors

NASA Technical Reports Server (NTRS)

Weiland, Karen J. R.; Wise, Michael L.; Smith, Gregory P.

1993-01-01

A variety of laser-induced fluorescence schemes were examined experimentally in atmospheric pressure flames to determine their use for sodium atom and salt detection in high-pressure, optically thick environments. Collisional energy transfer plays a large role in fluorescence detection. Optimum sensitivity, at the parts in 10 exp 9 level for a single laser pulse, was obtained with the excitation of the 4p-3s transition at 330 nm and the detection of the 3d-3p fluorescence at 818 nm. Fluorescence loss processes, such as ionization and amplified spontaneous emission, were examined. A new laser-induced atomization/laser-induced fluorescence detection technique was demonstrated for NaOH and NaCl. A 248-nm excimer laser photodissociates the salt molecules present in the seeded flames prior to atom detection by laser-induced fluorescence.

Short-wavelength out-of-band EUV emission from Sn laser-produced plasma

NASA Astrophysics Data System (ADS)

Torretti, F.; Schupp, R.; Kurilovich, D.; Bayerle, A.; Scheers, J.; Ubachs, W.; Hoekstra, R.; Versolato, O. O.

2018-02-01

We present the results of spectroscopic measurements in the extreme ultraviolet regime (7-17 nm) of molten tin microdroplets illuminated by a high-intensity 3 J, 60 ns Nd:YAG laser pulse. The strong 13.5 nm emission from this laser-produced plasma (LPP) is of relevance for next-generation nanolithography machines. Here, we focus on the shorter wavelength features between 7 and 12 nm which have so far remained poorly investigated despite their diagnostic relevance. Using flexible atomic code calculations and local thermodynamic equilibrium arguments, we show that the line features in this region of the spectrum can be explained by transitions from high-lying configurations within the Sn{}8+-Sn{}15+ ions. The dominant transitions for all ions but Sn{}8+ are found to be electric-dipole transitions towards the n = 4 ground state from the core-excited configuration in which a 4p electron is promoted to the 5s subshell. Our results resolve some long-standing spectroscopic issues and provide reliable charge state identification for Sn LPP, which could be employed as a useful tool for diagnostic purposes.

NaK 22Σ+ → 11Σ+ band optically pumped laser near 1.02 μm

NASA Astrophysics Data System (ADS)

Clark, B. K.; Luh, W. T.; Huennekens, J.

1989-08-01

Optically pumped laser emission has been observed on the NaK 2( A)1Σ+ → 1( X)1Σ+ electronic state transition. The emission occurs between 1.015 and 1.035 μm when a sodium-potassium heat-pipe oven is pumped with 695 745 nm pulsed dye laser radiation. The laser emission occurs on many ro-vibrational transitions without the use of cavity mirrors. However, the addition of a simple cavity increases both the number of observed lasing transitions and the amplitude of the emission on each line. We report our results for the dependence of the emission intensity on pump laser power, oven temperature, and buffer gas pressure.

Orthogonally superimposed laser-induced periodic surface structures (LIPSS) upon nanosecond laser pulse irradiation of SiO2/Si layered systems

NASA Astrophysics Data System (ADS)

Nürnberger, Philipp; Reinhardt, Hendrik M.; Kim, Hee-Cheol; Pfeifer, Erik; Kroll, Moritz; Müller, Sandra; Yang, Fang; Hampp, Norbert A.

2017-12-01

In this study we examined the formation of laser-induced periodic surface structures (LIPSS) on silicon (Si) in dependence on the thickness of silicon-dioxide (SiO2) on top. LIPSS were generated in air by linearly polarized ≈8 nanosecond laser pulses with a fluence per pulse of 2.41 J cm-2 at a repetition rate of 100 kHz. For SiO2 layers <80 nm, LIPSS oriented perpendicular to the laser polarization were obtained, but for SiO2 layers >120 nm parallel oriented LIPSS were observed. In both cases the periodicity was about 80-90% of the applied laser wavelength (λ0 = 532 nm). By variation of the SiO2 layer thickness in the range between 80 nm-120 nm, the dominating orientation changes. Even orthogonally superimposed LIPSS with a periodicity of only 60% of the laser wavelength were found. We show that the transition of the orientation direction of LIPSS is related to the penetration depth of surface plasmon polariton (SPP) fields into the oxide layer.

Diode laser operating on an atomic transition limited by an isotope ⁸⁷Rb Faraday filter at 780 nm.

PubMed

Tao, Zhiming; Hong, Yelong; Luo, Bin; Chen, Jingbiao; Guo, Hong

2015-09-15

We demonstrate an extended cavity Faraday laser system using an antireflection-coated laser diode as the gain medium and the isotope (87)Rb Faraday anomalous dispersion optical filter (FADOF) as the frequency selective device. Using this method, the laser wavelength works stably at the highest transmission peak of the isotope (87)Rb FADOF over the laser diode current from 55 to 140 mA and the temperature from 15°C to 35°C. Neither the current nor the temperature of the laser diode has significant influence on the output frequency. Compared with previous extended cavity laser systems operating at frequencies irrelevant to spectacular atomic transition lines, the laser system realized here provides a stable laser source with the frequency operating on atomic transitions for many practical applications.

A review of visible, near-IR, and mid-IR transitions in rare-earth doped glass waveguides for remote sensing and LIDAR

NASA Astrophysics Data System (ADS)

Jha, Animesh

2006-12-01

In the review article we explain the recent investigations on rare-earth doped glass and optical fibres for designing lasers which may be suitable for remote sensing and LIDAR applications. The paper explains the importance of engineering efficient lasing transitions in visible (480-650 nm) for generating UV lasers via one-stage harmonic generation. Besides visible transitions, we also demonstrate the transitions in near- and mid-IR via near-IR pumping scheme.

Excitation mechanism in a hollow cathode He-Kr ion laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hazama, J.; Arai, T.; Goto, M.

1995-12-31

Pulsed laser operation in the afterglow of a positive column He-Kr discharge on the 469.4 nm (6s{sup 4}P{sub 5/2} {yields} 5p{sup 4}P{sub 5/2}) transition of Kr(II) was observed for the first time by Dana and Laure`s. It appears that the upper level of Kr(II) laser line is populated by the second kind collisions between He 2{sup 3}S metastable atoms and ground state Kr ions. CW oscillations on Kr(II) transitions have been obtained in a hollow cathode discharge. In this work, we have estimated the excitation mechanism for the upper state of 469.4 nm laser line from the measurements of themore » decay of endlight intensity in the hollow cathode He-Kr discharge.« less

In-band-pumped Ho:KLu(WO4)2 microchip laser with 84% slope efficiency.

PubMed

Loiko, Pavel; Serres, Josep Maria; Mateos, Xavier; Yumashev, Konstantin; Kuleshov, Nikolai; Petrov, Valentin; Griebner, Uwe; Aguiló, Magdalena; Díaz, Francesc

2015-02-01

We report on a continuous-wave Ho:KLu(WO4)2 (KLuW) microchip laser with a record slope efficiency of 84%, the highest value among the holmium inband-pumped lasers, delivering 201 mW output power at 2105 nm. The Ho laser operating at room temperature on the (5)I8→(5)I7 transition is in-band-pumped by a diode-pumped Tm:KLuW microchip laser at 1946 nm. Ho:KLuW laser operation at 2061 and 2079 nm is also demonstrated with a maximum slope efficiency of 79%. The microchip laser generates an almost diffraction-limited output beam with a Gaussian profile and a M2<1.1. The laser performance of the Ng-cut Ho:KLuW crystal is very similar for pump light polarizations ‖Nm and Np. The positive thermal lens plays a key role in the laser mode stabilization and proper mode-matching. The latter, together with the low quantum defect under in-band-pumping (∼0.08), is responsible for the extraordinary high slope efficiency.

Constructing a Laser Stabilization System for a Parity Non-Conservation Experiment with Francium

NASA Astrophysics Data System (ADS)

Dehart, A. C.; Gwinner, Gerald; Kossin, Michael; Behr, John; Gorelov, Alexandre; Kalita, Mukut; Pearson, Matthew; Aubin, Seth; Gomez Garcia, Eduardo; Orozco, Luis

2017-04-01

We are developing an experiment at TRIUMF to test the Standard model at low energies by measuring Parity Non-Conservation (PNC) effects in francium. Current efforts include preparations to study the 7s - 8s electric dipole (E1) forbidden transition in francium at 507 nm under the influence of an electric field. Fr has no stable isotope; therefore to frequency-stabilize our laser at 507 nm, we are developing a laser stabilization system by using the Pound-Drever-Hall technique with a Fabry-Perot cavity made of Ultra Low Expansion Glass (ULE) as our stable frequency reference. The system will stabilize a 1014 nm laser, which will be frequency doubled to 507 nm, before sending the light to our cold and trapped francium sample. We will report on our recent experiences with the laser stabilization system. Supported by NSERC, NRC/TRIUMF, DOE, NSF, CONACYT, Fulbright, and U. of Manitoba.

Frequency stabilization of a 1083 nm fiber laser to {sup 4}He transition lines with optical heterodyne saturation spectroscopies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gong, W.; Peng, X., E-mail: xiangpeng@pku.edu.cn; Li, W.

2014-07-15

Two kinds of optical heterodyne saturation spectroscopies, namely, frequency modulation spectroscopy (FMS) and modulation transfer spectroscopy (MTS), are demonstrated for locking a fiber laser to the transition lines of metastable {sup 4}He atoms around 1083 nm. The servo-loop error signals of FMS and MTS for stabilizing laser frequency are optimized by studying the dependence of the peak-to-peak amplitude and slope on the optical power of pump and probe beams. A comparison of the stabilization performances of FMS/MTS and polarization spectroscopy (PS) is presented, which shows that MTS exhibits relatively superior performance with the least laser frequency fluctuation due to itsmore » flat-background dispersive signal, originated from the four-wave mixing process. The Allan deviation of the stabilized laser frequency is 5.4 × 10{sup −12}@100 s with MTS for data acquired in 1000 s, which is sufficiently applicable for fields like laser cooling, optical pumping, and optical magnetometry.« less

Picosecond rotationally resolved stimulated emission pumping spectroscopy of nitric oxide

NASA Astrophysics Data System (ADS)

Tanjaroon, Chakree; Reeve, Scott W.; Ford, Alan; Murry, W. Dean; Lyon, Kevin; Yount, Bret; Britton, Dan; Burns, William A.; Allen, Susan D.; Bruce Johnson, J.

2012-01-01

Stimulated emission pumping (SEP) experiments were performed on the nitric oxide molecule in a flow cell environment using lasers with pulse widths of 17-25 ps. A lambda excitation scheme, or ''pump-dump" arrangement, was employed with the pump laser tuned to the T 00 vibronic band origin ( λ=226.35(1)nm) of the A2Σ+( v' = 0, J') ← X2Π1/2( v″ = 0, J″) and the dump laser scanned from 246-248 nm within the A2Σ+( v' = 0, J') → X2Π1/2( v″ = 2, J″) transition. The rotationally resolved SEP spectra were measured by observing the total fluorescence within the A2Σ+( v' = 0, J') → X2Π1/2( v″ = 1, J″) transition between 235 nm and 237.2 nm while scanning the dump laser wavelengths. Multiple rotational states were excited due to the broad laser bandwidth. Measurements showed that the resolved rotational structure depended on the energy and bandwidth of the applied pump and dump laser pulses. Analysis of the observed fluorescence depletion signals yielded an average percent fluorescence depletion of about 19% when λ=226.35(1)nm and λ=247.91(1)nm. This value reflects the percent transfer of the NO population from the A2Σ+( V' = 0, J') excited electronic state to the X2Π1/2( v″ = 2, J″) ground electronic state. The maximum expected depletion is 50% in the limit of dump saturation. Selective excitation of NO at the bandhead provides good spectral discrimination from the background emission and noise and unambiguously confirms the identity of the emitter.

Heralded Quantum Gate between Remote Quantum Memories

DTIC Science & Technology

2009-06-25

emission fre- quency. Second, the geometrical modes from the two fibers are matched to better than 98% as characterized with laser light. Third, the...remains in the trap for several weeks. Doppler-cooling by laser light slightly red detuned from the 2S1=2 $ 2P1=2 transition at 369.5 nm localizes the ions...state decays to the metastable 2D3=2 level. This level is depopulated with a laser near 935.2 nm to maintain efficient cooling and state detection. We

Plasmonic enhancement of the vanadium dioxide phase transition induced by low-power laser irradiation

NASA Astrophysics Data System (ADS)

Ferrara, Davon W.; MacQuarrie, Evan R.; Diez-Blanco, Victor; Nag, Joyeeta; Kaye, Anthony B.; Haglund, Richard F.

2012-08-01

Nanocomposites consisting of gold nanoparticle (NP) arrays and vanadium dioxide (VO2) thin films are noteworthy for the tunability of both their thermal and optical properties. The localized surface plasmon resonance (LSPR) of the Au can be tuned when its dielectric environment is modulated by the semiconducting-to-metal phase transition (SMT) of the VO2; the LSPR itself can be altered by changing the shape of the NPs and the pitch of the NP array. In principle, then it should be possible to choose a combination of VO2 film and Au LSPR properties that maximizes the overall optical response of the nanocomposite. To demonstrate this effect, transient transmission measurements were conducted on lithographically fabricated arrays of Au NPs of diameter 140 nm, array spacing 350 nm, and covered with a 60 nm thick films of VO2 via pulsed laser deposition. Both Au::VO2 nanocomposites and bare VO2 film were irradiated with a shuttered 785 nm pump laser, and their optical response was probed at 1550 nm by a fixed-frequency diode laser. The Au::VO2 nanocomposite exhibited an increased effective absorption coefficient 1.5 times that of the plain film and required 37 % less laser power to induce the SMT. The time-dependent temperature rise in the film as a function of laser intensity was calculated from these measurements and compared with both analytic and finite-element models. Our results suggest that Au::VO2 nanocomposites may be useful in applications such as thermal-management coatings for energy efficient "smart" windows.

11 W narrow linewidth laser source at 780nm for laser cooling and manipulation of Rubidium

NASA Astrophysics Data System (ADS)

Sané, S. S.; Bennetts, S.; Debs, J. E.; Kuhn, C. C. N.; McDonald, G. D.; Altin, P. A.; Close, J. D.; Robins, N. P.

2012-04-01

We present a narrow linewidth continuous laser source with over 11 Watts of output power at 780nm, based on single-pass frequency doubling of an amplified 1560nm fibre laser with 36% efficiency. This source offers a combination of high power, simplicity, mode quality and stability. Without any active stabilization, the linewidth is measured to be below 10kHz. The fibre seed is tunable over 60GHz, which allows access to the D2 transitions in 87Rb and 85Rb, providing a viable high-power source for laser cooling as well as for large-momentum-transfer beamsplitters in atom interferometry. Sources of this type will pave the way for a new generation of high flux, high duty-cycle degenerate quantum gas experiments.

The suitability of barium monofluoride for laser cooling from ab initio study

NASA Astrophysics Data System (ADS)

Kang, Shuying; Kuang, Fangguang; Jiang, Gang; Du, Jiguang

2016-03-01

The feasibility of laser cooling the 138Ba19F molecule is performed using ab initio quantum chemistry. Three low-lying doublet electronic states X 2Σ+, A' 2Δ and A 2Π are determined by the multireference configuration-interaction (MRCI) method, where the spin-orbit coupling (SOC) effect is also taken into account in the electronic structure calculations. The computed spectroscopic constants and permanent dipole moments agree well with the available experimental data. The Franck-Condon factors of the A 2П → X 2Σ+ transition show highly diagonal dominance (f00 = 0.981, f11 = 0.940, f22 = 0.896) and the A 2П state has a radiative lifetime of τ = 37.8 ns, allowing for rapid laser cooling. Our calculation indicates that the laser-cooling scheme require only three lasers at 822 nm, 855 nm and 856 nm proceeded on the A 2П (ν‧) ← X 2Σ+ (ν‧‧) transitions. The appeared intervening state A' 2Δ between the X 2Σ+ and A 2П states is the main challenge for laser cooling this molecule. In fact, the calculated vibrational branching loss ratio to the intermediate A' 2Δ state is almost negligible at a level of η < 4.5 × 10-9. Thus, BaF is a promising laser-cooling candidate with a relatively simple laser-cooling scheme.

Tunable ultraviolet and blue light generation from Nd:YAB random laser bolstered by second-order nonlinear processes

NASA Astrophysics Data System (ADS)

Moura, André L.; Carreño, Sandra J. M.; Pincheira, Pablo I. R.; Fabris, Zanine V.; Maia, Lauro J. Q.; Gomes, Anderson S. L.; de Araújo, Cid B.

2016-06-01

Ultraviolet and blue light were obtained by nonlinear frequency conversion in a random laser (RL) based on Nd0.10Y0.90Al3(BO3)4 nanocrystalline powder. RL operation at 1062 nm, due to the 4F3/2 → 4I11/2 transition of neodymium ions (Nd3+), was achieved by exciting the Nd3+ with a tunable beam from 680 to 920 nm covering the ground state absorption transitions to the 4F9/2, (4F7/2,4S3/2), (4F5/2,2H9/2), and 4F3/2 states. Light from 340 to 460 nm was obtained via the second-harmonic generation of the excitation beam while tunable blue light, from 417 to 486 nm, was generated by self-sum-frequency mixing between the excitation beam and the RL emission.

Detection of the level of fluoride in the commercially available toothpaste using laser induced breakdown spectroscopy with the marker atomic transition line of neutral fluorine at 731.1 nm

NASA Astrophysics Data System (ADS)

Gondal, M. A.; Maganda, Y. W.; Dastageer, M. A.; Al Adel, F. F.; Naqvi, A. A.; Qahtan, T. F.

2014-04-01

Fourth harmonic of a pulsed Nd:YAG laser (wavelength 266 nm) in combination with high resolution spectrograph equipped with Gated ICCD camera has been employed to design a high sensitive analytical system. This detection system is based on Laser Induced Breakdown Spectroscopy and has been tested first time for analysis of semi-fluid samples to detect fluoride content present in the commercially available toothpaste samples. The experimental parameters were optimized to achieve an optically thin and in local thermo dynamic equilibrium plasma. This improved the limits of detection of fluoride present in tooth paste samples. The strong atomic transition line of fluorine at 731.102 nm was used as the marker line to quantify the fluoride concentration levels. Our LIBS system was able to detect fluoride concentration levels in the range of 1300-1750 ppm with a detection limit of 156 ppm.

One step beyond the electric dipole approximation: An experiment to observe the 5p → 6p forbidden transition in atomic rubidium

NASA Astrophysics Data System (ADS)

Ponciano-Ojeda, F.; Hernández-Gómez, S.; Mojica-Casique, C.; Ruiz-Martínez, E.; López-Hernández, O.; Colín-Rodríguez, R.; Ramírez-Martínez, F.; Flores-Mijangos, J.; Sahagún, D.; Jáuregui, R.; Jiménez-Mier, J.

2018-01-01

An advanced undergraduate experiment to study the 5 P 3 / 2 → 6 P 3 / 2 electric quadrupole transition in rubidium atoms is presented. The experiment uses two external cavity diode lasers, one operating at the D2 rubidium resonance line and the other built with commercial parts to emit at 911 nm. The lasers produce the 5 s → 5 p → 6 p excitation sequence in which the second step is the forbidden transition. Production of atoms in the 6 P 3 / 2 state is observed by detection of the 420 nm fluorescence that results from electric dipole decay into the ground state. Lines whose widths are significantly narrower than the Doppler width are used to study the hyperfine structure of the 6 P 3 / 2 state in rubidium. The spectra illustrate characteristics unique to electric dipole forbidden transitions, like the electric quadrupole selection rules; they are also used to show general aspects of two-color laser spectroscopy such as velocity selection and hyperfine pumping.

Analysis of unresolved transition arrays in XUV spectral region from highly charged lead ions produced by subnanosecond laser pulse

NASA Astrophysics Data System (ADS)

Wu, Tao; Higashiguchi, Takeshi; Li, Bowen; Arai, Goki; Hara, Hiroyuki; Kondo, Yoshiki; Miyazaki, Takanori; Dinh, Thanh-Hung; O'Reilly, Fergal; Sokell, Emma; O'Sullivan, Gerry

2017-02-01

Soft x-ray and extreme ultraviolet (XUV) spectra from lead (Pb, Z=82) laser-produced plasmas (LPPs) were measured in the 1.0-7.0 nm wavelength region employing a 150-ps, 1064-nm Nd:YAG laser with focused power densities in the range from 3.1×1013 W/cm2 to 1.4×1014 W/cm2. The flexible atomic code (FAC) and the Cowan's suite of atomic structure codes were applied to compute and explain the radiation properties of the lead spectra observed. The most prominent structure in the spectra is a broad double peak, which is produced by Δn=0, n=4-4 and Δn=1, n=4-5 transition arrays emitted from highly charged lead ions. The emission characteristics of Δn=1, n=4-5 transitions were investigated by the use of the unresolved transition arrays (UTAs) model. Numerous new spectral features generated by Δn=1, n=4-5 transitions in ions from Pb21+ to Pb45+ are discerned with the aid of the results from present computations as well as consideration of previous theoretical predictions and experimental data.

LED-pumped Alexandrite laser oscillator and amplifier

NASA Astrophysics Data System (ADS)

Pichon, Pierre; Blanchot, Jean-Philippe; Balembois, François; Druon, Frédéric; Georges, Patrick

2018-02-01

In this paper, we report the first LED-pumped transition-metal-doped laser oscillator and amplifier based on an alexandrite crystal (Cr3+:BeAl2O4). A Ce:YAG luminescent concentrator illuminated by blue LEDs is used to reach higher pump powers than with LEDs alone. The luminescent 200-mm-long-composit luminescent concentrator involving 2240 LEDs can delivers up to 268 mJ for a peak irradiance of 8.5 kW/cm2. In oscillator configuration, an LED-pumped alexandrite laser delivering an energy of 2.9 mJ at 748 nm in free running operation is demonstrated. In the cavity, we measured a double pass small signal gain of 1.28, in good agreement with numerical simulations. As amplifier, the system demonstrated to boost a CW Ti:sapphire laser by a factor of 4 at 750 nm in 8 passes with a large tuning range from 710 nm to 800 nm.

Compact fs ytterbium fiber laser at 1010 nm for biomedical applications.

PubMed

Kong, Cihang; Pilger, Christian; Hachmeister, Henning; Wei, Xiaoming; Cheung, Tom H; Lai, Cora S W; Huser, Thomas; Tsia, Kevin K; Wong, Kenneth K Y

2017-11-01

Ytterbium-doped fiber lasers (YDFLs) working in the near-infrared (NIR) spectral window and capable of high-power operation are popular in recent years. They have been broadly used in a variety of scientific and industrial research areas, including light bullet generation, optical frequency comb formation, materials fabrication, free-space laser communication, and biomedical diagnostics as well. The growing interest in YDFLs has also been cultivated for the generation of high-power femtosecond (fs) pulses. Unfortunately, the operating wavelengths of fs YDFLs have mostly been confined to two spectral bands, i.e., 970-980 nm through the three-level energy transition and 1030-1100 nm through the quasi three-level energy transition, leading to a spectral gap (990-1020 nm) in between, which is attributed to an intrinsically weak gain in this wavelength range. Here we demonstrate a high-power mode-locked fs YDFL operating at 1010 nm, which is accomplished in a compact and cost-effective package. It exhibits superior performance in terms of both short-term and long-term stability, i.e., <0.3% (peak intensity over 2.4 μs) and <4.0% (average power over 24 hours), respectively. To illustrate the practical applications, it is subsequently employed as a versatile fs laser for high-quality nonlinear imaging of biological samples, including two-photon excited fluorescence microscopy of mouse kidney and brain sections, as well as polarization-sensitive second-harmonic generation microscopy of potato starch granules and mouse tail muscle. It is anticipated that these efforts will largely extend the capability of fs YDFLs which is continuously tunable over 970-1100 nm wavelength range for wideband hyperspectral operations, serving as a promising complement to the gold-standard Ti:sapphire fs lasers.

Compact fs ytterbium fiber laser at 1010 nm for biomedical applications

PubMed Central

Kong, Cihang; Pilger, Christian; Hachmeister, Henning; Wei, Xiaoming; Cheung, Tom H.; Lai, Cora S. W.; Huser, Thomas; Tsia, Kevin. K.; Wong, Kenneth K. Y.

2017-01-01

Ytterbium-doped fiber lasers (YDFLs) working in the near-infrared (NIR) spectral window and capable of high-power operation are popular in recent years. They have been broadly used in a variety of scientific and industrial research areas, including light bullet generation, optical frequency comb formation, materials fabrication, free-space laser communication, and biomedical diagnostics as well. The growing interest in YDFLs has also been cultivated for the generation of high-power femtosecond (fs) pulses. Unfortunately, the operating wavelengths of fs YDFLs have mostly been confined to two spectral bands, i.e., 970-980 nm through the three-level energy transition and 1030-1100 nm through the quasi three-level energy transition, leading to a spectral gap (990-1020 nm) in between, which is attributed to an intrinsically weak gain in this wavelength range. Here we demonstrate a high-power mode-locked fs YDFL operating at 1010 nm, which is accomplished in a compact and cost-effective package. It exhibits superior performance in terms of both short-term and long-term stability, i.e., <0.3% (peak intensity over 2.4 μs) and <4.0% (average power over 24 hours), respectively. To illustrate the practical applications, it is subsequently employed as a versatile fs laser for high-quality nonlinear imaging of biological samples, including two-photon excited fluorescence microscopy of mouse kidney and brain sections, as well as polarization-sensitive second-harmonic generation microscopy of potato starch granules and mouse tail muscle. It is anticipated that these efforts will largely extend the capability of fs YDFLs which is continuously tunable over 970-1100 nm wavelength range for wideband hyperspectral operations, serving as a promising complement to the gold-standard Ti:sapphire fs lasers. PMID:29188091

Spectroscopy and lasing of Tm:SrMoO4 crystal near 1.5, 1.9, and 2.3-μm under 793-nm excitation

NASA Astrophysics Data System (ADS)

Šulc, Jan; Švejkar, Richard; Němec, Michal; Doroshenko, Maxim E.; Jelínková, Helena; Ivleva, Liudmila I.; Dunaeva, Elizaveta E.

2018-02-01

The spectroscopy properties and lasing of diode pumped Tm-doped strontium molybdate SrMoO4 single crystal were investigated at room temperature. The Tm:SrMoO4 crystal was grown by modified Stepanov method (2 wt.% of TmNbO4 in the melt). The tested Tm:SrMoO4 sample was cut from the grown crystal boule perpendicularly to growth direction 100. For spectroscopy and laser experiments 4.2mm thick plane-parallel face-polished plate (without AR coatings) was used. A fiber-coupled laser diode operating at wavelength 793nm was used for longitudinal Tm:SrMoO4 pumping which corresponds to 3H4 level excitation. Fluorescence spectra measurement showed strong emission in vicinity of 1.8 μm (3F4 -> 3H6 transition), and also significant emission close to wavelengths 1.45 μm (3H4 -> 3F4 transition) and 2.3 μm (3H4 -> 3H5 transition). The lasing was successfully reached for all these three transitions and output characteristics were measured. The pumping laser diode was operating in the pulsed regime with a low duty cycle. The 145mm long semi-hemispherical laser resonator consisted of flat pumping mirror (HT @ 0.79 μm) and curved (r = 150mm) output coupler. For each lasing transition the particular set of resonator mirrors was used to reach high reflexivity of pumping mirror and output coupler transmission 0.5% at laser operation wavelength. The obtained laser emission wavelengths were 1.95 μm, 1.45 & 1.49 μm, and 2.30 μm. In spite of low laser slope efficiency in respect to absorbed pumping power (0.45% for 3H4 -> 3F4 transition, 0.50% for 3F4 -> 3H6 transition and 0.83% for 3H4 -> 3H5 transition), results obtained are promising for further development of diode-pumped laser at 2.3 μm spectral region.

Apker Award Talk: Atomic Beam Measurement of the Indium 6p1 / 2 Scalar Polarizability

NASA Astrophysics Data System (ADS)

Augenbraun, Benjamin

2016-05-01

We report on the first measurement of the scalar polarizability of the indium 6p1 / 2 -excited state using two-step laser spectroscopy in an atomic beam. This is one in a series of precise atomic structure measurements by the Majumder lab at Williams College, which serve as stringent tests of abinitio calculation methods for three-valence-electron systems. We stabilize a laser to the indium 5p1 / 2 --> 6s1 / 2 410 nm transition and scan a second laser across the 6s1 / 2 --> 6p1 / 2 1343 nm transition. The two laser beams are overlapped and interact transversely with a collimated atomic beam of indium. Two-tone FM spectroscopy allows us to observe the small (< 1 part in 103) IR absorption, and characteristic sideband features in the RF-demodulated lineshape provide built-in frequency calibration. Application of DC electric fields up to 20 kV/cm give rise to Stark shifts of order 100 MHz. Because our group has previously measured the difference in polarizabilities within the 410 nm transition, we can determine the 6p1 / 2 polarizability with no loss of precision. Preliminary results are in excellent agreement with recent theoretical calculations and can be used to infer accurate values for the indium 6 p - 5 d matrix elements.

Stabilized 1762 nm Laser for Barium Ion Qubit Readout via Adiabatic Passage

NASA Astrophysics Data System (ADS)

Salacka, Joanna

2008-05-01

Trapped ions are one of the most promising candidates for the implementation of quantum computation. We are trapping single ions of Ba^137 to serve as our qubit, because the hyperfine structure of its ground state and its various visible-wavelength transitions make it favorable for quantum computation. The two hyperfine ground levels will serve as our |1> and |0> qubit states. The readout of the qubit will be accomplished by first selectively shelving the ion directly to the metastable 5D5/2 state using a 1762 nm narrow band fiber laser. Next, the cooling and repumping lasers are turned on and the fluorescence of the ion is measured. Since the 5D5/2 state is decoupled from the laser cooling transitions, the ion will remain dark when shelved. Thus if fluorescence is seen we know that the qubit was in the |0> state, and if no fluorescence is seen it was in the |1> state. The laser is actively stabilized to a temperature-controlled, high-finesse 1.76 um Zerodur optical cavity. The shelving to the 5D5/2 state is most efficiently achieved with adiabatic passage, which requires a smooth scan of the laser frequency across the transition resonance. To accomplish this, the laser frequency is modulated by an AOM driven by a smooth frequency sweep of adjustable amplitude and duration.

Characteristics of indium-gallium-nitride multiple-quantum-well blue laser diodes grown by MOCVD

NASA Astrophysics Data System (ADS)

Mack, M. P.; Abare, A. C.; Hansen, M.; Kozodoy, P.; Keller, S.; Mishra, U.; Coldren, L. A.; DenBaars, S. P.

1998-06-01

Room temperature (RT) pulsed operation of blue (420 nm) nitride-based multi-quantum well (MQW) laser diodes grown on c-plane sapphire substrates has been demonstrated. Atmospheric pressure MOCVD was used to grow the active region of the device which consisted of a 10 pair In 0.21Ga 0.79N (2.5 nm)/In 0.07Ga 0.93N (5 nm) InGaN MQW. Threshold current densities as low as 12.6 kA/cm 2 were observed for 10×1200 μm lasers with uncoated reactive ion etched (RIE) facets. The emission is strongly TE polarized and has a sharp transition in the far-field pattern above threshold. Laser diodes were tested under pulsed conditions lasted up to 6 h at room temperature.

Continuous-wave Nd:GYSGG laser at 1.1 μm

NASA Astrophysics Data System (ADS)

Lin, Hongyi; Liu, Hong; Huang, Xiaohua; Copner, Nigel; Sun, Dong

2018-02-01

We demonstrated a compact and simple continuous-wave (CW) Nd:GYSGG laser with triple-wavelength lines at 1105, 1107 and 1110 nm based on R2 → Y6, R1 → Y5 and R1 → Y6 of the 4F3/2 → 4I11/2 transition. The total output power of the triple-wavelength lines was 480 mW. Moreover, we obtained an efficient CW Nd:GYSGG laser at 1110 nm with the output power of 1560 mW at the pump power of 11.05 W. Those lines at 1058 and 1062 nm were suppressed completely by the simple output mirror of high transmission at 1.06 μm.

Multi-wavelength emission through self-induced second-order wave-mixing processes from a Nd3+ doped crystalline powder random laser

NASA Astrophysics Data System (ADS)

Moura, André L.; Jerez, Vladimir; Maia, Lauro J. Q.; Gomes, Anderson S. L.; de Araújo, Cid B.

2015-09-01

Random lasers (RLs) based on neodymium ions (Nd3+) doped crystalline powders rely on multiple light scattering to sustain laser oscillation. Although Stokes and anti-Stokes Nd3+ RLs have been demonstrated, the optical gain obtained up to now was possibly not large enough to produce self-frequency conversion. Here we demonstrate self-frequency upconversion from Nd3+ doped YAl3(BO3)4 monocrystals excited at 806 nm, in resonance with the Nd3+ transition 4I9/2 → 4F5/2. Besides the observation of the RL emission at 1062 nm, self-converted second-harmonic at 531 nm, and self-sum-frequency generated emission at 459 nm due to the RL and the excitation laser at 806 nm, are reported. Additionally, second-harmonic of the excitation laser at 403 nm was generated. These results exemplify the first multi-wavelength source of radiation owing to nonlinear optical effect in a Nd3+ doped crystalline powder RL. Contrary to the RLs based on dyes, this multi-wavelength light source can be used in photonic devices due to the large durability of the gain medium.

Stress assisted selective ablation of ITO thin film by picosecond laser

NASA Astrophysics Data System (ADS)

Farid, Nazar; Chan, Helios; Milne, David; Brunton, Adam; M. O'Connor, Gerard

2018-01-01

Fast selective pattering with high precession on 175 nm ITO thin film with IR ps lasers is investigated. Ablation parameters are optimized with detailed studies on the scribed depth, topography, and particle generation using AFM and SEM. A comparison of 10 and 150 ps laser revealed that the shorter pulse (10 ps) laser is more appropriate in selective and partial ablation; up to 20 nm resolution for controlled depth with multipulses having energy below the damage threshold is demonstrated. The experimental results are interpreted to involve stress assisted ablation mechanism for the 10 ps laser while thermal ablation along with intense melting occurs for 150 ps laser. The transition between these regimes is estimated to occur at approximately 30 ps.

Quasi-three level Nd:YLF fundamental and Raman laser operating under 872-nm and 880-nm direct diode pumping

NASA Astrophysics Data System (ADS)

Wetter, Niklaus U.; Bereczki, Allan; Paes, João. Pedro Fonseca

2018-02-01

Nd:YLiF4 is the gain material of choice whenever outstanding beam quality or a birefringent gain material is necessary such as in certain applications for terahertz radiation or dual-frequency mode-locking. However, for high power CW applications the material is hampered by a low thermal fracture threshold. This problem can be mitigated by special 2D pump set-ups or by keeping the quantum defect to a minimum. Direct pumping into the upper laser level of Nd:YLiF4 is usually performed at 880 nm. For quasi-three level laser emission at 908 nm, direct pumping at this wavelength provides a high quantum defect of 0.97, which allows for very high CW pump powers. Although the direct pumping transition to the upper laser state at 872 nm has a slightly smaller quantum defect of 0.96, its pump absorption cross section along the c-axis is 50% higher than at 880 nm, leading to a higher absorption efficiency. In this work we explore, for the first time to our knowledge, 908 nm lasing under 872 nm diode pumping and compare the results with 880 nm pumping for quasicw and cw operation. By inserting a KGW crystal in the cavity, Raman lines at 990 nm and 972 nm were obtained for the first time from a directly pumped 908 nm Nd:YLF fundamental laser for both quasi-cw and cw conditions.

Novel Flame-Based Synthesis of Nanowires for Multifunctional Application

DTIC Science & Technology

2015-05-13

referenced above, the laser fluence is appropriately low so that only a nanoplasma is created around the nanoparticle with no gas-phase breakdown or...and 501.428 nm corresponding to Ti (I) atomic emission lines [20] from the nanoparticle-induced nanoplasmas are observed. However, for 355 nm...Ren, Q. Yao, and C. K. Law, "Two-dimensional imaging of gas-to-particle transition in flames by laser-induced nanoplasmas ," Applied Physics Letters

Silicon carbide white light LEDs for solid-state lighting

NASA Astrophysics Data System (ADS)

Bet, Sachin; Quick, Nathaniel; Kar, Aravinda

2007-02-01

White light emitting diodes (LEDs) have been successfully fabricated for the first time in silicon carbide substrates (4H-SiC) using a novel laser doping technique. The donor-acceptor pair (DAP) recombination mechanism for luminescence has been used to tailor these LEDs. Chromium (Cr), which produces multiple acceptor sites per atom, and selenium which produces multiple donor sites per atom were successfully incorporated into SiC for the first time using laser doping. Aluminum (Al) and nitrogen (N) were also laser-doped into SiC. Green (521-575 nm) and blue (460-498 nm) wavelengths were observed due to radiative recombination transitions between donor-acceptors pairs of N-Cr and N-Al respectively, while a prominent violet (408 nm) wavelength was observed due to transitions from the nitrogen level to the valence band level. The red (698-738 nm) luminescence was mainly due to nitrogen excitons and other defect levels. This RGB combination produced a broadband white light spectrum extending from 380 to 900 nm. The color space tri-stimulus values were X = 0.3322, Y = 0.3320 and Z = 0.3358 as per 1931 CIE (International Commission on Illumination) for 4H-SiC corresponding to a color rendering index of 96.56; the color temperature of 5510 K is very close to average daylight (5500 K).

Frequency stabilized diode laser with variable linewidth at a wavelength of 404.7  nm.

PubMed

Rein, Benjamin; Walther, Thomas

2017-04-15

We report on a frequency stabilized laser system with a variable linewidth at a wavelength of 404.7 nm used as an incoherent repump on the 6P3₀↔7S3₁ transition in mercury. By directly modulating the laser diode current with Gaussian white noise, the laser linewidth can be broadened up to 68 MHz. A Doppler-free dichroic atomic vapor laser lock spectroscopy provides an error signal suitable for frequency stabilization even for the broadened laser. Without the need of an acousto-optic modulator for the linewidth tuning or lock-in technique for frequency stabilization, this laser system provides an inexpensive approach for an incoherent and highly efficient repumper in atomic experiments.

Single diode laser sensor for wide-range H2O temperature measurements.

PubMed

Gharavi, Mohammadreza; Buckley, Steven G

2004-04-01

A single diode laser absorption sensor (near 1477 nm) useful for simultaneous temperature and H2O concentration measurements is developed. The diode laser tunes approximately 1.2 cm(-1) over three H2O absorption transitions in each measurement. The line strengths of the transitions are measured over a temperature range from 468 to 977 K, based on high-resolution absorption measurements in a heated static cell. The results indicate that the selected transitions are suitable for sensitive temperature measurements in atmospheric pressure combustion systems using absorption line ratios. Comparing the results with HITRAN 96 data, it appears that these transitions will be sensitive over a wide range of temperatures (450-2000 K), suggesting applicability for combustion measurements.

Challenges Analyzing Gypsum on Mars by Raman Spectroscopy.

PubMed

Marshall, Craig P; Olcott Marshall, Alison

2015-09-01

Raman spectroscopy can provide chemical information about organic and inorganic substances quickly and nondestructively with little to no sample preparation, thus making it an ideal instrument for Mars rover missions. The ESA ExoMars planetary mission scheduled for launch in 2018 will contain a miniaturized Raman spectrometer (RLS) as part of the Pasteur payload operating with a continuous wave (CW) laser emitting at 532 nm. In addition, NASA is independently developing two miniaturized Raman spectrometers for the upcoming Mars 2020 rover mission, one of which is a remote (stand-off) Raman spectrometer that uses a pulse-gated 532 nm excitation system (SuperCam). The other is an in situ Raman spectrometer that employs a CW excitation laser emitting at 248.6 nm (SHERLOC). Recently, it has been shown with analyses by Curiosity that Gale Crater contains significantly elevated concentrations of transition metals such as Cr and Mn. Significantly, these transition metals are known to undergo fluorescence emission in the visible portion of the electromagnetic spectrum. Consequently, samples containing these metals could be problematic for the successful acquisition of fluorescence-free Raman spectra when using a CW 532 nm excitation source. Here, we investigate one analog environment, with a similar mineralogy and sedimentology to that observed in martian environments, as well as elevated Cr contents, to ascertain the best excitation wavelength to successfully collect fluorescence-free spectra from Mars-like samples. Our results clearly show that CW near-infrared laser excitation emitting at 785 nm is better suited to the collection of fluorescence-free Raman spectra than would be a CW laser emitting at 532 nm.

[Two-photon up-conversion fluorescence of a neodymium organic framework Nd(BTC)].

PubMed

Xu, Hui; Jin, Run-zhi; Wu, Chun-yang; Yang, Yu; Qian, Guo-dong

2008-08-01

In the present work, a neodymium organic framework Nd(BTC) was synthesized by the solvothermal reaction of Nd(NO3)3 x 5H2O and H3BTC (BTC = 1,3,5-benzenetricarboxylate) in mixed solvents of DMF, ethanol and water, and was identified by elemental analysis. This MOF complex was characterized using X-ray diffraction (XRD), thermogravimetry-differential scanning calorimetry (TGA-DSC) analysis, UV-visible absorption spectra and fluorescence spectra. This polycrystalline powder lost DMF and H2O when heated to 120 degrees C, then remained stable till the temperature reached 500 degrees C. Near infrared fluorescence at 1064 nm due to the 4 F3/2--> 4 I11/2 transition of Nd3+ ions was exhibited when excited by 808 nm laser beam. It was also been found that up-conversion fluorescence of Nd(BTC) peaked at about 450 nm due to 2 D5/2 -->4 I11/2 transition of Nd3+ ions can be observed under the excitation of a 580 nm laser line. The mechanism of the up-conversion fluorescence of Nd(BTC) at around 450 nm under the excitation of 580 nm laser can be ascribed to both excited-state absorption and energy transfer up-conversion. This result indicated that such MOF can be employed as an up-conversion luminescence material in many potential application areas such as bio-labeling and fluorescence image.

Toward Ultraintense Compact RBS Pump for Recombination 3.4 nm Laser via OFI

NASA Astrophysics Data System (ADS)

Suckewer, S.; Ren, J.; Li, S.; Lou, Y.; Morozov, A.; Turnbull, D.; Avitzour, Y.

In our presentation we overview progress we made in developing a new ultrashort and ultraintensive laser system based on Raman backscattering (RBS) amplifier /compressor from time of 10th XRL Conference in Berlin to present time of 11th XRL Conference in Belfast. One of the main objectives of RBS laser system development is to use it for pumping of recombination X-ray laser in transition to ground state of CVI ions at 3.4 nm. Using elaborate computer code the processes of Optical Field Ionization, electron energy distribution, and recombination were calculated. It was shown that in very earlier stage of recombination, when electron energy distribution is strongly non-Maxwellian, high gain in transition from the first excited level n=2 to ground level m=1 can be generated. Adding large amount of hydrogen gas into initial gas containing carbon atoms (e.g. methane, CH4) the calculated gain has reached values up to 150-200 cm-2 Taking into account this very encouraging result, we have proceed with arrangement of experimental setup. We will present the observation of plasma channels and measurements of electron density distribution required for generation of gain at 3.4 nm.

Laser Induced Fluorescence of Helium Ions in a Helicon Plasma

NASA Astrophysics Data System (ADS)

Compton, C. S.; Biloui, C.; Hardin, R. A.; Keesee, A. M.; Scime, E. E.; Boivin, R.

2003-10-01

The lack of a suitable Laser Induced Fluorescence (LIF) scheme for helium ions at visible wavelengths has prevented LIF from being employed in helium plasmas for measurements of ion temperature and bulk ion flow speeds. In this work, we will discuss our attempts to perform LIF of helium ions in a helicon source plasma using an infrared, tunable diode laser operating at 1012.36 nm. The infrared transition corresponds to excitation from the n = 4 level (4f ^2F) to the n = 5 (5g ^2G) level of singly ionized helium and therefore requires substantial electron temperatures (> 10 eV) to maintain an adequate ion population in the n = 4 state. Calculations using a steady state coronal model predict that the n = 4 state population will be 25% larger than the n = 5 population for our experimental conditions. The fluorescence decay from the n = 5 (5f ^2F) level of singly ionized helium level to the n = 3 (3d ^2D) level at 320.31 nm is monitored as the diode laser is swept through 10 GHz around the 1012.36 nm line. Note that the fluorescence emission requires a collisionally coupled transition between two different n = 5 quantum states. We will also present measurements of the emission intensities of both the 1012.36 nm and the 320.31 nm lines as a function of source neutral pressure, rf power, and plasma density. This work supported by the U.S. DoE EPSCoR Lab Partnership Program.

High-sensitivity remote detection of atmospheric pollutants and greenhouse gases at low ppm levels using near-infrared tunable diode lasers

NASA Astrophysics Data System (ADS)

Roy, Anirban; Upadhyay, Abhishek; Chakraborty, Arup Lal

2016-05-01

The concentration of atmospheric pollutants and greenhouse gases needs to be precisely monitored for sustainable industrial development and to predict the climate shifts caused by global warming. Such measurements are made on a continuous basis in ecologically sensitive and urban areas in the advanced countries. Tunable diode laser spectroscopy (TDLS) is the most versatile non-destructive technology currently available for remote measurements of multiple gases with very high selectivity (low cross-sensitivity), very high sensitivity (on the order of ppm and ppb) and under hazardous conditions. We demonstrate absolute measurements of acetylene, methane and carbon dioxide using a fielddeployable fully automated TDLS system that uses calibration-free 2f wavelength modulation spectroscopy (2f WMS) techniques with sensitivities of low ppm levels. A 40 mW, 1531.52 nm distributed feedback (DFB) diode laser, a 10 mW, 1650 nm DFB laser and a 1 mW, 2004 nm vertical cavity surface emitting laser (VCSEL) are used in the experiments to probe the P9 transition of acetylene, R4 transition of methane and R16 transition of carbon dioxide respectively. Data acquisition and on-board analysis comprises a Raspberry Pi-based embedded system that is controllable over a wireless connection. Gas concentration and pressure are simultaneously extracted by fitting the experimental signals to 2f WMS signals simulated using spectroscopic parameters obtained from the HITRAN database. The lowest detected concentration is 11 ppm for acetylene, 275 ppm for methane and 285 ppm for carbon dioxide using a 28 cm long single-pass gas cell.

Cryogenic Tm: YAG Laser in the Near Infrared

DTIC Science & Technology

2015-05-29

Applications Group. The focus of his work at Lincoln Laboratory has been solid-state lasers including microchip lasers , external-cavity diode lasers ...REPLACE THIS LINE WITH YOUR PAPER IDENTIFICATION NUMBER (DOUBLE-CLICK HERE TO EDIT) < Cryogenic Tm:YAG Laser in the Near Infrared* Tso Yee Fan...Senior Member, IEEE, Juan R. Ochoa, and Patricia A. Reed Abstract- Thulium laser operation on the 3H4 - 3H6 transition at 823 nm has been demonstrated

Silicon Based Colloidal Quantum Dot and Nanotube Lasers

DTIC Science & Technology

2013-03-01

carrier density is theoretically and experimentally derived to be inversely proportional to the diameter; (b) demonstration of InGaN/ GaN light emitting...diodes and GaN single nanowire photonic crystal laser on silicon characterized by a lasing transition at λ=371.3 nm with a linewidth of 0.55 nm. The...derived to be inversely proportional to the diameter; (b) demonstration of InGaN/ GaN light emitting diodes and GaN single nanowire photonic crystal

Single-photon cesium Rydberg excitation spectroscopy using 318.6-nm UV laser and room-temperature vapor cell.

PubMed

Wang, Jieying; Bai, Jiandong; He, Jun; Wang, Junmin

2017-09-18

We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S 1/2 ground state to nP 3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser, and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S 1/2 , F = 4 - 6P 3/2 , F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state. Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and linewidth influenced by lasers' Rabi frequency have been investigated. Fitting to energies of Cs nP 3/2 (n = 70 -100) states, the determined quantum defect is 3.56671(42). The demodulated spectra can also be employed as frequency references to stabilize the UV laser frequency to specific Cs Rydberg transition.

Simultaneous tri-wavelength laser operation at 916, 1086, and 1089 nm of diode-pumped Nd:LuVO4 crystal

NASA Astrophysics Data System (ADS)

Shen, Bingjun; Jin, Lihong; Zhang, Jiajia; Tian, Jian

2016-09-01

We report a diode-pumped continuous-wave tri-wavelength Nd:LuVO4 laser operating at 916, 1086, and 1089 nm. A theoretical analysis has been introduced to determine the threshold conditions for simultaneous tri-wavelength laser operation. Using a T-shaped cavity, we realized efficient tri-wavelength operation at 4F3/2  →  4I9/2 and 4F3/2  →  4I11/2 transitions for Nd:LuVO4 crystal, simultaneously. The maximum output power was 2.8 W, which included 916, 1086, and 1089 nm, and the optical conversion efficiency was 15.1%. To our knowledge, this is the first work that realizes simultaneous tri-wavelength Nd:LuVO4 laser operation.

Upconversion emission study of Er{sup 3+} doped CaMoO{sub 4} phosphor

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sinha, Shriya, E-mail: Shriya.sinha6@gmail.com; Mahata, Manoj Kumar; Kumar, Kaushal

2016-05-06

The infrared to visible upconversion emission in Er{sup 3+} doped CaMoO{sub 4} phosphor has been investigated upon 980 nm diode laser excitation. The X-ray diffraction analysis reveals well crystalline nature and tetragonal phase structure of the prepared phosphor annealed at 800 °C. The Er{sup 3+} doped CaMoO{sub 4} phosphor has shown intense green upconversion emission upon 980 nm didode laser excitation. The green emission bands at 530 nm and 552 nm corresponds to the {sup 2}H{sub 11/2}→{sup 4}I{sub 15/2} and {sup 4}S{sub 3/2}→{sup 4}I{sub 15/2} electronic transitions, respectively of Er{sup 3+} ion. The very weak red emission band around 656more » nm is assigned to the {sup 4}F{sub 9/2}→{sup 4}I{sub 15/2} transition of Er{sup 3+} ion. The CIE color coordinate exhibits the emission color in intense green region, indicating the use of present phosphor in display device applications.« less

Highly-efficient mid-infrared CW laser operation in a lightly-doped 3 at.% Er:SrF2 single crystal.

PubMed

Su, Liangbi; Guo, Xinsheng; Jiang, Dapeng; Wu, Qinghui; Qin, Zhipeng; Xie, Guoqiang

2018-03-05

3 at.% Er:SrF 2 laser crystals with high optical quality were successfully grown using the temperature gradient technique (TGT). The intense mid-infrared emission was observed around 2.7 μm with excitation by a 970 nm LD. Based on the Judd-Ofelt theory, the emission cross-sections of the 4 I 13/2 - 4 I 11/2 transition were calculated by using the Fuchtbauer-Ladenburg (FL) method. Efficient continuous-wave laser operation at 2.8 µm was achieved with the lightly-doped 3 at.% Er:SrF 2 crystal pumped by a 970 nm laser diode. The laser output power reached up to 1.06 W with a maximum slope efficiency of 26%.

Collison-Induced Absorption of Oxygen Molecule as Studied by High Sensitivity Spectroscopy

NASA Astrophysics Data System (ADS)

Kashihara, Wataru; Shoji, Atsushi; Kawai, Akio

2017-06-01

Oxygen dimol is transiently generated when two oxygen molecules collide. At this short period, the electron clouds of molecules are distorted and some forbidden transition electronic transitions become partially allowed. This transition is called CIA (Collision-induced absorption). There are several CIA bands appearing in the spectral region from UV to near IR. Absorption of solar radiation by oxygen dimol is a small but significant part of the total budget of incoming shortwave radiation. However, a theory predicting the lineshape of CIA is still under developing. In this study, we measured CIA band around 630 nm that is assigned to optical transition, a^{1}Δ_{g}(v=0):a^{1}Δ_{g}(v=0)-X^{3}Σ_{g}^{-}(v=0):X^{3}Σ_{g}^{-}(v=0) of oxygen dimol. CRDS(Cavity Ring-down Spectroscopy) was employed to measure weak absorption CIA band of oxygen. Laser beam around 630 nm was generated by a dye laser that was pumped by a YAG Laser. Multiple reflection of the probe light was performed within a vacuum chamber that was equipped with two high reflective mirrors. We discuss the measured line shape of CIA on the basis of collision pair model.

Broadband infrared light-emitting patterns in optical glass by laser-induced nanostructuring of NiO-doped alkali-gallium germanosilicates.

PubMed

Lotarev, S V; Lipatiev, A S; Golubev, N V; Ignat'eva, E S; Malashkevich, G E; Mudryi, A V; Priseko, Y S; Lorenzi, R; Paleari, A; Sigaev, V N

2013-02-15

In this Letter, we show functionalization of NiO-doped 7.5Li(2)O·2.5Na(2)O·20Ga(2)O(3)·35SiO(2)·35GeO(2) glass by space-selective nanocrystallization via exposure to the focused beam of a pulsed copper vapor laser (510.6 and 578.2 nm) at temperature close to the glass transition point (570°C). Irradiated areas drastically change their color, caused by electronic transitions of Ni(2+) dopant ions, without any alteration of the optical quality. Importantly, irradiated regions acquire broadband infrared luminescence (centered at about 1400 nm and possessing 400 nm effective bandwidth) typical of Ni(2+) ions in crystalline environment, and by positive change of refractive index (more than 10(-3)). Spectroscopic and diffractometric data of the irradiated regions indeed resemble those previously observed in thermally nanocrystallized glass, with Ni(2+) ions embedded in γ-Ga(2)O(3) nanocrystals. The results demonstrate the possibility of laser writing nanocrystallized multifunction patterns in germanosilicate glasses for the fabrication of active integrated devices.

Laser excitation dynamics of argon metastables generated in atmospheric pressure flows by microwave frequency microplasma arrays

NASA Astrophysics Data System (ADS)

Rawlins, W. T.; Galbally-Kinney, K. L.; Davis, S. J.; Hoskinson, A. R.; Hopwood, J. A.

2014-03-01

The optically pumped rare-gas metastable laser is a chemically inert analogue to diode-pumped alkali (DPAL) and alkali-exciplex (XPAL) laser systems. Scaling of these devices requires efficient generation of electronically excited metastable atoms in a continuous-wave electric discharge in flowing gas mixtures at atmospheric pressure. This paper describes initial investigations of the use of linear microwave micro-discharge arrays to generate metastable rare-gas atoms at atmospheric pressure in optical pump-and-probe experiments for laser development. Power requirements to ignite and sustain the plasma at 1 atm are low, <30 W. We report on the laser excitation dynamics of argon metastables, Ar (4s, 1s5) (Paschen notation), generated in flowing mixtures of Ar and He at 1 atm. Tunable diode laser absorption measurements indicate Ar(1s5) concentrations near 3 × 1012 cm-3 at 1 atm. The metastables are optically pumped by absorption of a focused beam from a continuous-wave Ti:S laser, and spectrally selected fluorescence is observed with an InGaAs camera and an InGaAs array spectrometer. We observe the optical excitation of the 1s5-->2p9 transition at 811.5 nm and the corresponding laser-induced fluorescence on the 2p10-->1s5 transition at 912.3 nm; the 2p10 state is efficiently populated by collisional energy transfer from 2p9. Using tunable diode laser absorption/gain spectroscopy, we observe small-signal gains of ~1 cm-1 over a 1.9 cm path. We also observe stable, continuous-wave laser oscillation at 912.3 nm, with preliminary optical efficiency ~55%. These results are consistent with efficient collisional coupling within the Ar(4s) manifold.

Nanometer-scale characterization of laser-driven plasmas, compression, shocks and phase transitions, by coherent small angle x-ray scattering

NASA Astrophysics Data System (ADS)

Kluge, Thomas

2015-11-01

Combining ultra-intense short-pulse and high-energy long-pulse lasers, with brilliant coherent hard X-ray FELs, such as the Helmholtz International Beamline for Extreme Fields (HIBEF) under construction at the HED Instrument of European XFEL, or MEC at LCLS, holds the promise to revolutionize our understanding of many High Energy Density Physics phenomena. Examples include the relativistic electron generation, transport, and bulk plasma response, and ionization dynamics and heating in relativistic laser-matter interactions, or the dynamics of laser-driven shocks, quasi-isentropic compression, and the kinetics of phase transitions at high pressure. A particularly promising new technique is the use of coherent X-ray diffraction to characterize electron density correlations, and by resonant scattering to characterize the distribution of specific charge-state ions, either on the ultrafast time scale of the laser interaction, or associated with hydrodynamic motion. As well one can image slight density changes arising from phase transitions inside of shock-compressed high pressure matter. The feasibility of coherent diffraction techniques in laser-driven matter will be discussed. including recent results from demonstration experiments at MEC. Among other things, very sharp density changes from laser-driven compression are observed, having an effective step width of 10 nm or smaller. This compares to a resolution of several hundred nm achievedpreviously with phase contrast imaging. and on behalf of HIBEF User Consortium, for the Helmholtz International Beamline for Extreme Fields at the European XFEL.

Bidirectional current triggering in planar devices based on serially connected VO₂ thin films using 965 nm laser diode.

PubMed

Kim, Jihoon; Park, Kyongsoo; Kim, Bong-Jun; Lee, Yong Wook

2016-08-08

By incorporating a 965 nm laser diode, the bidirectional current triggering of up to 30 mA was demonstrated in a two-terminal planar device based on serially connected vanadium dioxide (VO₂) thin films grown by pulsed laser deposition. The bidirectional current triggering was realized by using the focused beams of laser pulses through the photo-thermally induced phase transition of VO₂. The transient responses of laser-triggered currents were also investigated when laser pulses excited the device at a variety of pulse widths and repetition rates of up to 4.0 Hz. A switching contrast between off- and on-state currents was obtained as ~8333, and rising and falling times were measured as ~39 and ~29 ms, respectively, for 50 ms laser pulses.

Structure, spectroscopic properties and laser performance of Nd:YNbO4 at 1066 nm

NASA Astrophysics Data System (ADS)

Ding, Shoujun; Peng, Fang; Zhang, Qingli; Luo, Jianqiao; Liu, Wenpeng; Sun, Dunlu; Dou, Renqin; Sun, Guihua

2016-12-01

We have demonstrated continuous wave (CW) laser operation of Nd:YNbO4 crystal at 1066 nm for the first time. A maximum output power of 1.12 W with the incident power of 5.0 W is successfully achieved corresponding to an optical-to-optical conversion efficiency of 22.4% and a slope efficiency of 24.0%. The large absorption cross section (8.7 × 10-20 cm2) and wide absorption band (6 nm) at around 808 nm indicates the good pumping efficiency by laser diodes (LD). The small emission cross section (29 × 10-20 cm2) and relative long lifetime of the 4F3/2 → 4I11/2 transition indicates good energy storage capacity of Nd:YNbO4. Moreover, the raw materials of Nd:YNbO4 are stable, thus, it can grow high-quality and large-size by Czochralski (CZ) method. Therefore the Nd:YNbO4 crystal is a potentially new laser material suitable for LD pumping.

Kinetics of UV laser radiation defects in high performance glasses

NASA Astrophysics Data System (ADS)

Natura, U.; Feurer, T.; Ehrt, D.

2000-05-01

High purity fluoride phosphate glasses are attractive candidates as UV transmitting materials. The calculated values for the ultraviolet resonance wavelength are comparable with those of pure silica glass or fluoride single crystal CaF2. The formation of radiation-induced defect centers leads to additional absorption bands in the VUV-UV-vis range. The damage and the healing behavior by lamps and lasers are investigated in dependence on phosphate content and the content of impurities, mainly transition metals. Experiments were carried out using pulsed lasers with a duration of femto- and nanoseconds at a wavelength of 248 nm. The initial slope of the induced absorption shows a nonlinear dependence on the pulse energy density. Resonant and non-resonant two-photon mechanisms were observed. Two-photon-absorption coefficients at 248 nm for samples with different phosphate contents were measured. Models of the kinetics of the radiation-induced defects were developed. The inclusion of energy transfer was necessary to explain the difference in the damage behavior for nanosecond (248 nm, 193 nm) and femtosecond (248 nm) laser pulses.

Development of a broadband reflectivity diagnostic for laser driven shock compression experiments

DOE PAGES

Ali, S. J.; Bolme, C. A.; Collins, G. W.; ...

2015-04-16

Here, a normal-incidence visible and near-infrared shock wave optical reflectivity diagnostic was constructed to investigate changes in the optical properties of materials under dynamic laser compression. Documenting wavelength- and time-dependent changes in the optical properties of laser-shock compressed samples has been difficult, primarily due to the small sample sizes and short time scales involved, but we succeeded in doing so by broadening a series of time delayed 800-nm pulses from an ultrafast Ti:sapphire laser to generate high-intensity broadband light at nanosecond time scales. This diagnostic was demonstrated over the wavelength range 450–1150 nm with up to 16 time displaced spectramore » during a single shock experiment. Simultaneous off-normal incidence velocity interferometry (velocity interferometer system for any reflector) characterized the sample under laser-compression and also provided an independent reflectivity measurement at 532 nm wavelength. The shock-driven semiconductor-to-metallic transition in germanium was documented by the way of reflectivity measurements with 0.5 ns time resolution and a wavelength resolution of 10 nm.« less

Spectroscopy and laser action of the "red perylimide dye" in various solvents

NASA Astrophysics Data System (ADS)

Gvishi, R.; Reisfeld, R.; Burshtein, Z.

1993-10-01

Optical properties of the red perylimide laser dye in various solvents are studied. The absorption spectrum exhibits two main bands, in the ranges 480-600 and 400-460 nm, due to the S 0-S 1 and S 0-S 2 transition. The fluorescence spectrum is a mirror image of the S 0-S 1 absorption (shift of ˜ 30-50 nm). The Stokes shift increases with solvent polarity. Such dye-solvent interactions are compared to theoretical predictions. The fluorescence quantum yields approaches unity in all the solvents studied. Laser tunability around 30 nm was obtained each time, covering the spectral range 580-640 nm. This interval is important for medical applications in photodynamic therapy and fluorescence diagnostics. The laser threshold energy varied from 0.35 mJ/pulse in cyclohexane to 1.87 mJ/pulse in methanol, and the slope efficiency from about 6.6% in methanol to 14% in xylenes. The laser output was stable for several hours of operation under an average pump energy of about 20 mJ/pulse at 1 Hz repetition rate, without flow.

Determination of phosphorus in steel by the combined technique of laser induced breakdown spectrometry with laser induced fluorescence spectrometry

NASA Astrophysics Data System (ADS)

Kondo, Hiroyuki; Hamada, Naoya; Wagatsuma, Kazuaki

2009-09-01

Laser induced breakdown spectrometry (LIBS) combined with laser induced fluorescence spectrometry (LIFS) has been applied for detection of trace-level phosphorus in steel. The plasma induced by irradiation of Nd:YAG laser pulse for ablation was illuminated by the 3rd harmonic of Ti:Sapphire laser tuned to one of the resonant lines for phosphorus in the wavelength region of 253-256 nm. An excitation line for phosphorus was selected to give the highest signal-to-noise ratio. Fluorescence signals, P213.62 and P214.91 nm, were observed with high selectivity at the contents as low as several tens µg g - 1 . Fluorescence intensities were in a good linear correlation with the contents. Fluorescence intensity ratio of a collisionally assisted line (213.62 nm) to a direct transition line (214.91 nm) was discussed in terms of the analytical conditions and experimental results were compared with a calculation based on rate equations. Since the fluorescence signal light in the wavelength range longer than 200 nm can be transmitted relatively easily, even through fiber optics of moderate length, LIBS/LIFS would be a versatile technique in on-site applications for the monitoring of phosphorus contents in steel.

An ultra-stable optical frequency standard for telecommunication purposes based upon the 5S1/2 → 5D5/2 two-photon transition in rubidium

NASA Astrophysics Data System (ADS)

Terra, Osama; Hussein, Hatem

2016-02-01

In this study, we report the development of a frequency standard for optical fiber communication applications based on a two-photon transition in rubidium at 385.2 THz. This standard kills two birds with one stone in the sense it is capable of providing us with two highly stable serviceable wavelengths at 778.1 and 1556.2 nm. In this system, we exploit the narrow line-width of a fiber laser emitting at 1556.2 nm in conjunction with an erbium-doped fiber amplifier to generate a sufficient second harmonic laser beam at 778.1 nm in a periodically polled lithium niobate waveguide mixer in order to probe and frequency-lock the laser to the 5S1/2 ( F g = 3)-5D5/2 ( F e = 5) hyperfine two-photon transition component in 85Rb. The metrological performance of the standard is evaluated with the aid of an optical frequency comb synthesizer. Allan variance measurement shows a stability of 4 × 10-12 at 1 s (limited by the comb stability), reaching a floor of 6.8 × 10-13 at 1000 s. After correction of all the major systematic frequency shifts including the light shift, the absolute frequency is found to be 385 285 142 374.0 (5.0) kHz. Moreover, the absolute frequencies of most of the hyperfine components of the 5S1/2-5D5/2 transition of the two naturally existing rubidium isotopes are measured using a femtosecond frequency comb synthesizer after stabilizing a laser on each component.

Laser-excited luminescence and absorption study of mixed valence for K 2Pt(CN) 4—K 2Pt(CN) 6 crystals

NASA Astrophysics Data System (ADS)

Kasi Viswanath, A.; Smith, Wayne L.; Patterson, H.

1982-04-01

Crystals of K 2Pt(CN) 6 doped with Pt(CN) 2-4 show an absorption band at 337 nm which is assigned as a mixed-valence (MV) transition from Pt (II) to Pt(IV). From a Hush model analysis, the absorption band is interpreted to be class II in the Day—Robin scheme. When the MV band is laser excited at 337 nm, emmision is observed from Pt(CN) 2-4 clusters.

Tailoring transition-metal hydroxides and oxides by photon-induced reactions

DOE PAGES

Niu, Kai -Yang; Fang, Liang; Ye, Rong; ...

2016-10-18

Controlled synthesis of transition-metal hydroxides and oxides with earth-abundant elements have attracted significant interest because of their wide applications, for example as battery electrode materials or electrocatalysts for fuel generation. Here, we report the tuning of the structure of transition-metal hydroxides and oxides by controlling chemical reactions using an unfocused laser to irradiate the precursor solution. A Nd:YAG laser with wavelengths of 532 nm or 1064 nm was used. The Ni 2+, Mn 2+, and Co 2+ ion-containing aqueous solution undergoes photo-induced reactions and produces hollow metal-oxide nanospheres (Ni 0.18Mn 0.45Co 0.37O x) or core–shell metal hydroxide nanoflowers ([Ni 0.15Mnmore » 0.15Co 0.7(OH) 2](NO 3) 0.2•H 2O), depending on the laser wavelengths. We propose two reaction pathways, either by photo-induced redox reaction or hydrolysis reaction, which are responsible for the formation of distinct nanostructures. As a result, the study of photon-induced materials growth shines light on the rational design of complex nanostructures with advanced functionalities.« less

Transitions of the type 2s-2p in oxygenlike Y, Zr, and Nb

NASA Technical Reports Server (NTRS)

Behring, W. E.; Brown, C. M.; Feldman, U.; Seely, J. F.; Reader, J.

1986-01-01

Transitions of the type 2s-2p in the oxygenlike ions Y XXXII, Zr XXXIII, and Nb XXXIV were identified in spectra recorded at the University of Rochester's Omega laser facility. Solid targets were spherically irradiated by 24 beams of frequency-tripled (351-nm) Nd-glass laser radiation. The spectra were photographed with a 3-m grazing-incidence spectrograph. The identified transitions of the oxygenlike ions are in the range 30 to 73 A. The wavelengths for the magnetic-dipole transitions within the 2s2p4 ground configurations of these ions are predicted from the experimental energy levels.

Development of a see-through hollow cathode discharge lamp for (Li/Ne) optogalvanic studies

NASA Astrophysics Data System (ADS)

Saini, V. K.; Kumar, P.; Sarangpani, K. K.; Dixit, S. K.; Nakhe, S. V.

2017-09-01

Development of a demountable and see-through hollow cathode (HC) discharge lamp suitable for optogalvanic (OG) spectroscopy is described. The design of the HC lamp is simple, compact, and inexpensive. Lithium, investigated rarely by the OG method, is selected for cathode material as its isotopes are important for nuclear industry. The HC lamp is characterized electrically and optically for discharge oscillations free OG effect. Strong OG signals of lithium as well as neon (as buffer gas) are produced precisely upon copper vapor laser pumped tunable dye laser irradiation. The HC lamp is capable of generating a clean OG resonance spectrum in the available dye laser wavelength scanning range (627.5-676 nm) obtained with 4-(Dicyanomethylene)-2-methyl-6-(4-dimethylaminostyryl)-4H-pyran dye. About 28 resonant OG lines are explicitly observed. Majority of them have been identified using j-l coupling scheme and assigned to the well-known neon transitions. One line that corresponds to wavelength near about 670.80 nm is assigned to lithium and resolved for its fine (2S1/2 → 2P1/2, 3/2) transitions. These OG transitions allow 0.33 cm-1 accuracy and can be used to supplement the OG transition data available from other sources to calibrate the wavelength of a scanning dye laser with precision at atomic levels.

Development of a see-through hollow cathode discharge lamp for (Li/Ne) optogalvanic studies.

PubMed

Saini, V K; Kumar, P; Sarangpani, K K; Dixit, S K; Nakhe, S V

2017-09-01

Development of a demountable and see-through hollow cathode (HC) discharge lamp suitable for optogalvanic (OG) spectroscopy is described. The design of the HC lamp is simple, compact, and inexpensive. Lithium, investigated rarely by the OG method, is selected for cathode material as its isotopes are important for nuclear industry. The HC lamp is characterized electrically and optically for discharge oscillations free OG effect. Strong OG signals of lithium as well as neon (as buffer gas) are produced precisely upon copper vapor laser pumped tunable dye laser irradiation. The HC lamp is capable of generating a clean OG resonance spectrum in the available dye laser wavelength scanning range (627.5-676 nm) obtained with 4-(Dicyanomethylene)-2-methyl-6-(4-dimethylaminostyryl)-4H-pyran dye. About 28 resonant OG lines are explicitly observed. Majority of them have been identified using j-l coupling scheme and assigned to the well-known neon transitions. One line that corresponds to wavelength near about 670.80 nm is assigned to lithium and resolved for its fine ( 2 S 1/2 → 2 P 1/2, 3/2 ) transitions. These OG transitions allow 0.33 cm -1 accuracy and can be used to supplement the OG transition data available from other sources to calibrate the wavelength of a scanning dye laser with precision at atomic levels.

NaK (DX) stimulated emission in the visible

NASA Astrophysics Data System (ADS)

Dinev, S. G.; Hadjichristov, G. B.

1990-12-01

Using optical pumping in the blue 450-470 nm and green 510.6 nm, we have observed molecular laser action in the D→X electronic transition of the heteronuclear NaK molecule. Pumping, emission and competing mechanisms are discussed together with the energy balance of the system.

Analysis of Optogalvanic Transients at 621.7 nm, 633.4 nm and 640.2 nm of Neon in a Discharge Plasma Fitted with a Monte Carlo Mathematical Model.

NASA Astrophysics Data System (ADS)

Ogungbemi, Kayode; Han, Xianming; Blosser, Micheal; Misra, Prabhakar; LASER Spectroscopy Group Collaboration

2014-03-01

Optogalvanic transitions have been recorded and fitted for 1s5 - 2p7\\ (621.7 nm), 1s5 - 2p8 (633.4 nm) and 1s5 - 2p9 (640.2 nm) transitions of neon in a Fe-Ne hollow cathode plasma discharge as a function of current (2-19 mA) and time evolution (0-50 microsec). The optogalvanic waveforms have been fitted to a Monte carlo mathematical model. The variation in the excited population of neon is governed by the rate of collision of the atoms involving the common metastable state (1s5) for the three transitions investigated. The concomitant changes in amplitudes and intensities of the optogalvanic signal waveforms associated with these transitions have been studied rigorously and the fitted parameters obtained using the Monte Carlo algorithm to help better understand the physics of the hollow cathode discharge. Thanks to Laser Spectroscopy group in Physics and Astronomy Dept. Howard University Washington DC.

Tunable Q-switched erbium doped fiber laser based on metal transition oxide saturable absorber and refractive index characteristic of multimode interference effects

NASA Astrophysics Data System (ADS)

Mohammed, D. Z.; Khaleel, Wurood Abdulkhaleq; Al-Janabi, A. H.

2017-12-01

Ferro-oxide (Fe3O4) nanoparticles were used as a saturable absorber (SA) for a passively Q-switched erbium doped fiber laser (EDFL) with ring cavity. The Q-switching operation was achieved at a pump threshold of 80 mW. The proposed fiber laser produces stable pulses train of repetition rate ranging from 25 kHz to 80 kHz as the pump power increases from threshold to 342 mW. The minimum recorded pulse width was 2.7 μs at 342 mW. The C-band tunability operation was performed using single mode-multimode-single mode fiber (SM-MM-SM) structure. The laser exhibited a total tuning range of 7 nm, maximum sensitivity of 106.9 nm, optical signal to noise ratio (OSNR) of 38 dB and 3-dB linewidth of 0.06 nm.

Observation of the 5 p3 /2→6 p3 /2 electric-dipole-forbidden transition in atomic rubidium using optical-optical double-resonance spectroscopy

NASA Astrophysics Data System (ADS)

Ponciano-Ojeda, F.; Hernández-Gómez, S.; López-Hernández, O.; Mojica-Casique, C.; Colín-Rodríguez, R.; Ramírez-Martínez, F.; Flores-Mijangos, J.; Sahagún, D.; Jáuregui, R.; Jiménez-Mier, J.

2015-10-01

Direct evidence of excitation of the 5 p3 /2→6 p3 /2 electric-dipole-forbidden transition in atomic rubidium is presented. The experiments were performed in a room-temperature rubidium cell with continuous-wave external cavity diode lasers. Optical-optical double-resonance spectroscopy with counterpropagating beams allows the detection of the nondipole transition free of Doppler broadening. The 5 p3 /2 state is prepared by excitation with a laser locked to the maximum F cyclic transition of the D2 line, and the forbidden transition is produced by excitation with a 911 nm laser. Production of the forbidden transition is monitored by detection of the 420 nm fluorescence that results from decay of the 6 p3 /2 state. Spectra with three narrow lines (≈13 MHz FWHM) with the characteristic F -1 , F , and F +1 splitting of the 6 p3 /2 hyperfine structure in both rubidium isotopes were obtained. The results are in very good agreement with a direct calculation that takes into account the 5 s →5 p3 /2 preparation dynamics, the 5 p3 /2→6 p3 /2 nondipole excitation geometry, and the 6 p3 /2→5 s1 /2 decay. The comparison also shows that the electric-dipole-forbidden transition is a very sensitive probe of the preparation dynamics.

Extreme ultraviolet emission spectra of Gd and Tb ions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kilbane, D.; O'Sullivan, G.

2010-11-15

Theoretical extreme ultraviolet emission spectra of gadolinium and terbium ions calculated with the Cowan suite of codes and the flexible atomic code (FAC) relativistic code are presented. 4d-4f and 4p-4d transitions give rise to unresolved transition arrays in a range of ions. The effects of configuration interaction are investigated for transitions between singly excited configurations. Optimization of emission at 6.775 nm and 6.515 nm is achieved for Gd and Tb ions, respectively, by consideration of plasma effects. The resulting synthetic spectra are compared with experimental spectra recorded using the laser produced plasma technique.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Razhev, A M; Kargapol'tsev, E S; Churkin, D S

Results of an experimental study of the influence of a gas mixture (laser active medium) composition on an output energy and total efficiency of gas-discharge excimer lasers on ArF* (193 nm), KrCl* (222 nm), KrF* (248 nm) and XeCl* (308 nm) molecules operating without a buffer gas are presented. The optimal ratios of gas components (from the viewpoint of a maximum output energy) of an active medium are found, which provide an efficient operation of laser sources. It is experimentally confirmed that for gas-discharge excimer lasers on halogenides of inert gases the presence of a buffer gas in an activemore » medium is not a necessary condition for efficient operation. For the first time, in two-component gas mixtures of repetitively pulsed gas-discharge excimer lasers on electron transitions of excimer molecules ArF*, KrCl*, KrF* and XeCl*, the pulsed energy of laser radiation obtained under pumping by a transverse volume electric discharge in a low-pressure gas mixture without a buffer gas reached up to 170 mJ and a high pulsed output power (of up to 24 MW) was obtained at a FWHM duration of the KrF-laser pulse of 7 ns. The maximal total efficiency obtained in the experiment with two-component gas mixtures of KrF and XeCl lasers was 0.8%. (lasers)« less

Size-controlled synthesis of transition metal nanoparticles through chemical and photo-chemical routes

NASA Astrophysics Data System (ADS)

Tangeysh, Behzad

The central objective of this work is developing convenient general procedures for controlling the formation and stabilization of nanoscale transition metal particles. Contemporary interest in developing alternative synthetic approaches for producing nanoparticles arises in large part from expanding applications of the nanomaterials in areas such as catalysis, electronics and medicine. This research focuses on advancing the existing nanoparticle synthetic routes by using a new class of polymer colloid materials as a chemical approach, and the laser irradiation of metal salt solution as a photo-chemical method to attain size and shape selectivity. Controlled synthesis of small metal nanoparticles with sizes ranging from 1 to 5nm is still a continuing challenge in nanomaterial synthesis. This research utilizes a new class of polymer colloid materials as nano-reactors and protective agents for controlling the formation of small transition metal nanoparticles. The polymer colloid particles were formed from cross-linking of dinegatively charged metal precursors with partially protonated poly dimethylaminoethylmethacrylate (PDMAEMA). Incorporation of [PtCl6]2- species into the colloidal particles prior to the chemical reduction was effectively employed as a new strategy for synthesis of unusually small platinum nanoparticles with narrow size distributions (1.12 +/-0.25nm). To explore the generality of this approach, in a series of proof-of-concept studies, this method was successfully employed for the synthesis of small palladium (1.4 +/-0.2nm) and copper nanoparticles (1.5 +/-0.6nm). The polymer colloid materials developed in this research are pH responsive, and are designed to self-assemble and/or disassemble by varying the levels of protonation of the polymer chains. This unique feature was used to tune the size of palladium nanoparticles in a small range from 1nm to 5nm. The procedure presented in this work is a new convenient room temperature route for synthesis of small nanoparticles, and its application can be extended to the formation of other transition metals and alloy nanoparticles. This research also focuses on developing new photo-chemical routes for controlling the size and shape of the nanoparticles through high-intensity ultra-fast laser irradiation of metal salt solution. One of the core objectives of this work is to explore the special capabilities of shaped laser pulses in formation of metal nanoparticles through irradiation of the solutions by using simultaneous spatial and temporal focusing (SSTF). Femtosecond laser irradiation has not yet been widely applied for nanoparticle synthesis, and offers new regimes of energy deposition for synthesis of nanomaterials. Photo-reduction of aqueous [AuCl4]- solution to the gold nanoparticles (AuNPs) has been applied as a model process for optimizing the experimental procedures, and evaluating the potential of shaped laser pulses in the synthesis of AuNPs. Systematic manipulation of the laser parameters and experimental conditions provided effective strategies to control the size of Au nanoparticles in strong laser fields. Varying the concentration of polyethylene glycol (PEG45) as a surfactant effectively tuned the size of AuNPs from 3.9 +/-0.7nm to 11.0 +/-2.4nm, and significantly increased the rate of Au(III) reduction during irradiation. Comparative studies revealed the capability of shaped laser pulses in the generation of smaller and more uniform AuNPs (5.8 +/-1.1nm) relative to the other conventional laser irradiation methods (7.2 +/-2.9nm). Furthermore, a new laser-assisted approach has been developed for selective formation of triangular Au nanoplates in the absence of any surfactant molecule. This method relies on rapid energy deposition by using shaped, ultra-intense laser pulses to generate Au seeds in aqueous [AuCl4]- solution, and the slow post-irradiation reduction of un-reacted [AuCl4]- species by using H2O2 as a mild reducing agent. Variation of the laser irradiation-time was found as an effective strategy to tune the morphology of Au nanomaterials from nanospheres to triangular nanoplates. The surfactant-free Au nanoplates produced in this research can be readily functionalized with a variety of target molecules or surfactants for desirable applications such as biomedicine. The concept of rapid laser processing followed by in situ chemical reduction can be expanded as a general methodology for high-yield production of nanomaterials, and provides a series of new laser dependent parameters for controlling the nanoparticle formation.

Studies on pulsed optogalvanic effect in Eu/Ne hollow cathode discharge.

PubMed

Saini, V K; Kumar, P; Dixit, S K; Nakhe, S V

2014-07-01

The optogalvanic (OG) effect has been observed in a Eu/Ne hollow cathode discharge lamp using pulsed laser irradiation. An OG spectrum is recorded in dye laser wavelength region 574–602 nm using a boxcar-averager. In total 41 atomic lines are observed. Of these, 38 lines are assigned to neon transitions. Two lines observed corresponding to wavelengths 576.519 and 601.815 nm are assigned to europium transitions; (4f 7 6s 2 , S 8 7/2 →4f 7 6s6p , zP 6 7/2 ) and (4f 7 6s 2 , S 8 7/2 →4f 7 6s6p , zP 8 9/2 ), respectively, and the remaining line at 582.475 nm could not be assigned. The effect of the discharge current on europium as well as neon OG signals is also studied. At moderate discharge current values, an extra positive peak is observed in neon OG signal for the transition (1s 5 →2p 2 ) at 588.189 nm, which is explained by Penning-ionization process using the quasi-resonant energy transfer interactions between excited neon and europium atoms lying in 2p 2 and D 10 9/2 states, respectively.

Continuous-wave yellow-green laser at 0.56  μm based on frequency doubling of a diode-end-pumped ceramic Nd:YAG laser.

PubMed

Yao, Wenming; Gao, Jing; Zhang, Long; Li, Jiang; Tian, Yubing; Ma, Yufei; Wu, Xiaodong; Ma, Gangfei; Yang, Jianming; Pan, Yubai; Dai, Xianjin

2015-06-20

We present what is, to the best of our knowledge, the first report on yellow-green laser generation based on the frequency doubling of the 1.1 μm transitions in Nd:YAG ceramics. By employing an 885 nm diode laser as the end-pumping source and a lithium triborate crystal as the frequency doubler, the highest continuous wave output powers of 1.4, 0.5, and 1.1 W at 556, 558, and 561 nm are achieved, respectively. These result in optical-to-optical efficiencies of 6.9%, 2.5%, and 5.4% with respect to the absorbed pump power, respectively.

An auto-locked diode laser system for precision metrology

NASA Astrophysics Data System (ADS)

Beica, H. C.; Carew, A.; Vorozcovs, A.; Dowling, P.; Pouliot, A.; Barron, B.; Kumarakrishnan, A.

2017-05-01

We present a unique external cavity diode laser system that can be auto-locked with reference to atomic and molecular spectra. The vacuum-sealed laser head design uses an interchangeable base-plate comprised of a laser diode and optical elements that can be selected for desired wavelength ranges. The feedback light to the laser diode is provided by a narrow-band interference filter, which can be tuned from outside the laser cavity to fineadjust the output wavelength in vacuum. To stabilize the laser frequency, the digital laser controller relies either on a pattern-matching algorithm stored in memory, or on first or third derivative feedback. We have used the laser systems to perform spectroscopic studies in rubidium at 780 nm, and in iodine at 633 nm. The linewidth of the 780-nm laser system was measured to be ˜500 kHz, and we present Allan deviation measurements of the beat note and the lock stability. Furthermore, we show that the laser system can be the basis for a new class of lidar transmitters in which a temperature-stabilized fiber-Bragg grating is used to generate frequency references for on-line points of the transmitter. We show that the fiber-Bragg grating spectra can be calibrated with reference to atomic transitions.

Alternative laser system for cesium magneto-optical trap via optical injection locking to sideband of a 9-GHz current-modulated diode laser.

PubMed

Diao, Wenting; He, Jun; Liu, Zhi; Yang, Baodong; Wang, Junmin

2012-03-26

By optical injection of an 852-nm extended-cavity diode laser (master laser) to lock the + 1-order sideband of a ~9-GHz-current-modulated diode laser (slave laser), we generate a pair of phase-locked lasers with a frequency difference up to ~9-GHz for a cesium (Cs) magneto-optical trap (MOT) with convenient tuning capability. For a cesium MOT, the master laser acts as repumping laser, locked to the Cs 6S₁/₂ (F = 3) - 6P₃/₂ (F' = 4) transition. When the + 1-order sideband of the 8.9536-GHz-current-modulated slave laser is optically injection-locked, the carrier operates on the Cs 6S₁/₂ (F = 4) - 6P₃/₂ (F' = 5) cooling cycle transition with -12 MHz detuning and acts as cooling/trapping laser. When carrying a 9.1926-GHz modulation signal, this phase-locked laser system can be applied in the fields of coherent population trapping and coherent manipulation of Cs atomic ground states.

Amplified stimulated emission in the NaK(D-X) band by high power copper vapor laser pumping

NASA Astrophysics Data System (ADS)

Dinev, S. G.; Hadjicristov, G. B.; Marazov, O.

1991-04-01

Using a 10 W copper vapor laser we have studied a stimulated emission at 520-570 nm in the D-X electronic transition of the NaK heteronuclear molecule. The influence of the cavity configuration on the bound-bound stimulated lines is considered.

Amplified stimulated emission in the NaK( D→ X) band by high power copper vapor laser pumping

NASA Astrophysics Data System (ADS)

Dinev, S. G.; Hadjichristov, G. B.; Marazov, O.

1991-04-01

Using a 10 W copper vapor laser we have studied a stimulated emission at 520 570 nm in the D→ X electronic transition of the NaK heteronuclear molecule. The influence of the cavity configuration on the bound-bound stimulated lines is considered.

Towards Precision Measurement of the 21S0-31D2 Two-Photon Transition in Atomic Helium

NASA Astrophysics Data System (ADS)

Huang, Yi-Jan; Guan, Yu-Chan; Suen, Te-Hwei; Wang, Li-Bang; Shy, Jow-Tsong

2017-04-01

We intend to accurately measure the frequency for 2S-3D two-photon transition and to deduce the 2S ionization energy to an accuracy below 100 kHz from the theoretical calculation of the 3D state. In this talk, we present a precision measurement of the 21S0 -31D2 two-photon transition in atomic helium at 1009 nm. A master oscillator power amplifier (MOPA) is seeded by an external cavity diode laser (ECDL) is constructed to generate more than 700 mW laser power with TEM00 beam profile at 1009 nm. To observe the two-photon transition, a helium cell is placed inside a power enhancement optical cavity and the helium atoms at 21S metastable level are prepared by a pulsed RF discharge and monitor the 668 nm 31D2 to 21P1 fluorescence after RF discharge is turned off . The absolute frequency metrology of the ECDL is carried out by an Er-fiber optical frequency comb (OFC). The two-photon spectrum is obtained by tuning the repetition frequency of the OFC. The 21S0-31D2 frequency is determined to be 594414291.967 (80) MHz in He-4. More results will be presented at the annual meeting.

Diode-Laser Absorption Sensor for Line-of-Sight Gas Temperature Distributions

NASA Astrophysics Data System (ADS)

Sanders, Scott T.; Wang, Jian; Jeffries, Jay B.; Hanson, Ronald K.

2001-08-01

Line-of-sight diode-laser absorption techniques have been extended to enable temperature measurements in nonuniform-property flows. The sensing strategy for such flows exploits the broad wavelength-scanning abilities ( >1.7 nm ~ 30 cm-1 ) of a vertical cavity surface-emitting laser (VCSEL) to interrogate multiple absorption transitions along a single line of sight. To demonstrate the strategy, a VCSEL-based sensor for oxygen gas temperature distributions was developed. A VCSEL beam was directed through paths containing atmospheric-pressure air with known (and relatively simple) temperature distributions in the 200 -700 K range. The VCSEL was scanned over ten transitions in the R branch of the oxygen A band near 760 nm and optionally over six transitions in the P branch. Temperature distribution information can be inferred from these scans because the line strength of each probed transition has a unique temperature dependence; the measurement accuracy and resolution depend on the details of this temperature dependence and on the total number of lines scanned. The performance of the sensing strategy can be optimized and predicted theoretically. Because the sensor exhibits a fast time response ( ~30 ms) and can be adapted to probe a variety of species over a range of temperatures and pressures, it shows promise for industrial application.

High energy efficient solid state laser sources

NASA Technical Reports Server (NTRS)

Byer, Robert L.

1987-01-01

Diode-laser-pumped solid-state laser oscillators and nonlinear processes were investigated. A new generation on nonplanar oscillator was fabricated, and it is anticipated that passive linewidths will be pushed to the kilohertz regime. A number of diode-pumped laser transitions were demonstrated in the rod configuration. Second-harmonic conversion efficiencies as high as 15% are routinely obtained in a servo-locked external resonant doubling crystal at 15 mW cw input power levels at 1064 nm.

Ho:YAG Single Crystal Fiber: Fabrication and Optical Characterization

DTIC Science & Technology

2014-06-16

between the 5I8 and 5I7 energy levels. The results verified the absorption peaks suitable for in- band direct pumping at 1908 nm and 1932 nm with the...Efficient high-power Ho:YAG laser directly in- band pumped by a GaSb -based laser diode stack at 1.9 μm,” Appl. Phys. B 106(2), 315–319 (2012). 21. M...characterized for its optical absorption and emission properties involving transitions between the 5I8 and 5I7 energy levels. The results verified

Optical modulation of quantum cascade laser with optimized excitation wavelength.

PubMed

Yang, Tao; Chen, Gang; Tian, Chao; Martini, Rainer

2013-04-15

The excitation wavelength for all-optical modulation of a 10.6 μm mid-infrared (MIR) quantum cascade laser (QCL) was varied in order to obtain maximum modulation depth. Both amplitude and wavelength modulation experiments were conducted at 820 nm and 1550 nm excitation respectively, whereby the latter matches the interband transition in the QCL active region. Experimental results show that for continuous-wave mode-operated QCL, the efficiency of free carrier generation is doubled under 1550 nm excitation compared with 820 nm excitation, resulting in an increase of the amplitude modulation index from 19% to 36%. At the same time, the maximum wavelength shift is more than doubled from 1.05 nm to 2.80 nm. Furthermore, for the first time to our knowledge, we demonstrated the optical switching of a QCL operated in pulse mode by simple variation of the excitation wavelength.

Investigation of terbium in the ferroelectric crystal, gadolinium molybdate, as a potential laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Crouch, J.E.

A preliminary non-stimulated study of the laser host combination Gd(2 - x)Tb(x)(MoO4)3 is made. The host material, gadolinium molybdate (GMO), is a ferroelectric/ferroelastic crystal. An investigation of temperature and external electric field affects on the absorption and fluorescence of the crystal did not produce any unusual results. The terbium ion, Tb(3+), peak cross section in GMO for the 5D sub 4 to 7F sub 5 transition is 10 x 10 to the minus twenty first power sq. cm. at 300K. The wavelength of this four level laser transition is 543 nm. (GRA)

Saturated fluorescence method for determination of atomic transition probabilities: Application to the Ar i 430.0-nm (1s4-3p8) transition and the lifetime determination of the upper level

NASA Astrophysics Data System (ADS)

Hirabayashi, A.; Okuda, S.; Nambu, Y.; Fujimoto, T.

1987-01-01

We have developed a new method for determination of atomic transition probabilities based on laser-induced-fluorescence spectroscopy (LIFS). In the method one produces a known population of atoms in the upper level under investigation and relates it to an observed absolute line intensity. We have applied this method to the argon 430.0-nm line (1s4-3p8): In an argon discharge plasma the 1s5-level population and spatial distribution are determined by the self-absorption method combined with LIFS under conditions where the 3p8-level population is much lower than that of the 1s5 level. When intense laser light of 419.1 nm (1s5-3p8) irradiates the plasma and saturates the 3p8-level population, the produced 3p8-level population and its alignment can be determined from the 1s5-level parameters as determined above, by solving the master equation on the basis of broad-line excitation. By comparing the observed absolute fluorescence intensity of the 430.0-nm line with the above population, we have determined the transition probability to be A=(3.94+/-0.60)×105 s-1. We also determined the 3p8-level lifetime by LIFS. Several factors which might affect the measurement are discussed. The result is τ=127+/-10 ns.

Laser-Based Monitoring of CH4, CO2, NH3, and H2S in Animal Farming—System Characterization and Initial Demonstration

PubMed Central

Jaworski, Piotr; Nikodem, Michał

2018-01-01

In this paper, we present a system for sequential detection of multiple gases using laser-based wavelength modulation spectroscopy (WMS) method combined with a Herriot-type multi-pass cell. Concentration of hydrogen sulfide (H2S), methane (CH4), carbon dioxide (CO2), and ammonia (NH3) are retrieved using three distributed feedback laser diodes operating at 1574.5 nm (H2S and CO2), 1651 nm (CH4), and 1531 nm (NH3). Careful adjustment of system parameters allows for H2S sensing at single parts-per-million by volume (ppmv) level with strongly reduced interference from adjacent CO2 transitions even at atmospheric pressure. System characterization in laboratory conditions is presented and the results from initial tests in real-world application are demonstrated. PMID:29425175

Laser cooling of BH and GaF: insights from an ab initio study.

PubMed

Gao, Yu-feng; Gao, Tao

2015-04-28

The feasibility of laser cooling BH and GaF is investigated using ab initio quantum chemistry. The ground state X (1)Σ(+) and first two excited states (3)Π and (1)Π of BH and GaF are calculated using the multireference configuration interaction (MRCI) level of theory. For GaF, the spin-orbit coupling effect is also taken into account in the electronic structure calculations at the MRCI level. Calculated spectroscopic constants for BH and GaF show good agreement with available theoretical and experimental results. The highly diagonal Franck-Condon factors (BH: f00 = 0.9992, f11 = 0.9908, f22 = 0.9235; GaF: f00 = 0.997, f11 = 0.989, f22 = 0.958) for the (1)Π (v' = 0-2) → X (1)Σ(+) (v = 0-2) transitions in BH and GaF are determined, which are found to be in good agreement with the theoretical and experimental data. Radiative lifetime calculations of the (1)Π (v' = 0-2) state (BH: 131, 151, and 187 ns; GaF: 2.26, 2.36, and 2.48 ns) are found to be short enough for rapid laser cooling. The proposed laser cooling schemes that drive the (1)Π (v' = 0) → X (1)Σ(+) (v = 0) transition use just one laser wavelength λ00 (BH: 436 nm, GaF: 209 nm). Though the cooling wavelength of GaF is deep in the UVC, a frequency quadrupled Ti:sapphire laser (189-235 nm) could be capable of generating useful quantities of light at this wavelength. The present results indicate that BH and GaF are two good choices of molecules for laser cooling.

Compact lasing system at 13.5-nm to ground state of LiIII at 2Hz

NASA Astrophysics Data System (ADS)

Goltsov, A. Y.; Korobkin, D.; Nam, C. H.; Suckewer, Szymon

1997-11-01

The recent results of the demonstration of the lasing action at 13.5 nm in transition to ground state of LiIII at 2 Hz repetition rate using two lasers is being presented in this paper. A gain length of GL approximately equals 5.5 was measured in the 5 mm long, 0.3 mm diameter, LiF microcapillary using a 50 mJ, 250 fsec UV laser beam. The initial plasma was created in the microcapillary by a low power, relatively long pulse Nd/YAG laser. In order to shed light on observed unusually high efficiency of the ionization of the atoms in microcapillaries, the subpicosecond UV laser beam transmissions through the plasma in microcapillaries were measured. Strong dependence of the beam transmission on the delay time between inial plasma formation with the Nd/YAG laser and the sub-picosecond UV laser was recorded. The final part of the paper discusses some necessary conditions for an extension of the present results towards the shorter wavelength lasers with an emphasis on the presently conducted experiments at Princeton University for the generation gain at 4.8 nm in BV.

Development of a laser induced breakdown spectrometer for detection of toxic elements in cosmetic products

NASA Astrophysics Data System (ADS)

Maganda, Yasin Wandhami

In this research work we developed a highly sensitive analytical Laser Induced Breakdown Spectrometer to detect toxic elements in commercially available cosmetic products. These products are frequently used by many all over the world, therefore there is an increasing demand to determine concentration levels of toxic elements present in them because they cause dangerous diseases and most of them are highly carcinogenic and life threatening. Laser Induced Breakdown Spectroscopy (LIBS) was applied for spectroscopic analysis of cosmetic products such as tooth paste, synthetic hair dye, kohl eyeliners and talcum powder samples. These samples were purchased from the local market within the kingdom of Saudi Arabia. The LIBS method is based on spectroscopic analysis of plasma resulting from the interaction of a high power pulsed laser radiations with a sample medium. In order to improve the sensitivity of the spectrometer, the dependence of the LIBS signal intensity and plasma parameters such as temperature (T) and electron density (ne) on gate/time delay, laser fluence and wavelength of the excitation source for plasma generated under ambient conditions were studied. During this work Nd: YAG lasers having 266nm, 532 nm and 1064 nm wavelengths operating in Q-switch mode were used as the excitation sources in combination with a spectrograph having a gated ICCD camera. Boltzmann plots and stark broadening for the recorded spectral lines were used to estimate the plasma temperature and electron density respectively. Temporal evolution of the plasma temperature and electron density showed a t-2 dependence. On the other hand plasma temperature and electron density increased with increase in laser fluence but leveled off at higher fluencies. It is worth noting that in both cases 266 nm and 1064 nm excitation wavelengths consistently had the highest and lowest values respectively. Therefore a 266 nm wavelength Nd: YAG laser excitation source was selected to develop a highly sensitive Laser Induced Breakdown spectrometer to detect and quantify the fluoride (F), lead (Pb) and chromium (Cr) content in commercially available toothpaste, synthetic hair dye, kohl eyeliners and talcum powder samples. The experimental parameters such as gate/ delays and laser fluencies were optimized to achieve an optically thin and in local thermodynamic equilibrium plasma (L.T.E) which improved the limit of detection of our spectrometer. The choice of the parameters was validated using the Mcwhirter criterion. For fluoride detection in the toothpaste samples, a strong atomic transition line of fluorine at 731.102 nm was used as the marker line. The LIBS system was able to detect fluoride concentration levels in the range of 1300 - 1750 ppm with a detection limit of 156ppm.In the synthetic hair dye, chromium was detected using a strong atomic transition of chromium (Cr) at a wavelength 427.5 nm as the spectral marker line and the spectrometer with a detection limit of 1.2 ppm was able to detect chromium concentration levels in the range of 5-11 ppm. These results achieved with our LIBS system were compared with those obtained using a standard detection method such as ICP-MS. The results obtained are in excellent agreement with ICP-MS. Lead (Pb) and Chromium (Cr) in kohl were detected using atomic transitions at wavelengths of 405.7 nm and 425.4 nm respectively as the spectral marker lines. The system was calibrated for these toxic metals and it was able to detect Lead and Chromium in the range of 5-14 ppm and 4-9 ppm with detection limits of 1ppm and 2 ppm respectively. The LIBS results were compared with those obtained using ICP-MS and were in good agreement yielding a relative accuracy in the range 0.05-0.3 which is acceptable. Lead (Pb) and Chromium (Cr) levels in talcum powder samples were detected and quantified using strong transitions at wavelengths of 405.7 nm and 425.4 nm respectively. The LIBS system detected lead and chromium in the range of 15-17 ppm and 23-29 ppm with limits of detection of 1.96 ppm and 1.72 ppm respectively. The concentration levels of fluoride, lead and chromium detected using our LIBS system exceeded the permissible limits set by the Environmental agency and other regulatory organization and hence frequent use of such cosmetic products can be hazardous to human health. The LIBS spectrometer developed through this research work can be applied for analysis of many other samples like pharmaceutical, polymers, iron, volcanic eruption and geological samples for mineral quantification.

980-nm diode laser and fiber optic resectoscope in endourological surgery

NASA Astrophysics Data System (ADS)

Cecchetti, Walter; Guazzieri, Stefano; Tasca, Andrea; Dal Bianco, M.; Zattoni, Filiberto; Pagano, Francesco

1996-12-01

The 980 nm Ceralas D50 diode laser, produces homogeneous lesions on tissues of different nature. In our endourological tests we used the Ceralas D50 coupled with Comeg 24 ch laser resectoscope, and we treated 22 patients: n.5 bladder cancers, n.3 uretero pelvic junction obstructions, with hydronephrosis, n.3 urethra stenosis, n1 ureter stenosis, n.4 multiple upper tract transitional cell carcinomas, n.6 BPH treatments with VLAP modalities. Using the 1000 micrometers delivery fibers with different shaped tips, we obtained a bloodless sharp cut and easily vaporizations with minimum carbonizations, with power output in the range of 8-12 W, and 18-24W for VLAP.

Study of Mn laser ablation in methane atmosphere

NASA Astrophysics Data System (ADS)

Krstulović, N.; Labazan, I.; Milošević, S.

2006-02-01

Laser ablation of Mn target in vacuum and in the presence of CH4 was studied under 308 nm laser irradiation. Time-resolved emission using gated detection and scanning monochromator and absorption using the cavity ring-down spectroscopy were used to study vaporized plume. In the CH4 atmosphere we observed transitions identified as C2 and MnH bands, while these spectral features were not detected in emission spectra. This is a clear evidence of importance in combining both spectroscopic techniques in laser vaporized plume study.

High-pulse energy supercontinuum laser for high-resolution spectroscopic photoacoustic imaging of lipids in the 1650-1850 nm region.

PubMed

Dasa, Manoj Kumar; Markos, Christos; Maria, Michael; Petersen, Christian R; Moselund, Peter M; Bang, Ole

2018-04-01

We propose a cost-effective high-pulse energy supercontinuum (SC) source based on a telecom range diode laser-based amplifier and a few meters of standard single-mode optical fiber, with a pulse energy density as high as ~25 nJ/nm in the 1650-1850 nm regime (factor >3 times higher than any SC source ever used in this wavelength range). We demonstrate how such an SC source combined with a tunable filter allows high-resolution spectroscopic photoacoustic imaging and the spectroscopy of lipids in the first overtone transition band of C-H bonds (1650-1850 nm). We show the successful discrimination of two different lipids (cholesterol and lipid in adipose tissue) and the photoacoustic cross-sectional scan of lipid-rich adipose tissue at three different locations. The proposed high-pulse energy SC laser paves a new direction towards compact, broadband and cost-effective source for spectroscopic photoacoustic imaging.

Interband and intraband electron kinetics in non-thermal warm dense gold

NASA Astrophysics Data System (ADS)

Brennan Brown, Shaughnessy; Chen, Zhijiang; Curry, Chandra; Hering, Philippe; Hoffmann, Matthias C.; Ng, Andrew; Reid, Matthew; Tsui, Ying Y.; Glenzer, Siegfried H.

2015-11-01

Single-state warm dense matter may be produced via isochoric heating of thin metal foils using ultrafast high-power lasers. Previous experiments have confirmed that electron temperatures exceed ion temperatures during the initial picoseconds following excitation; however, electron kinetics in non-thermal states preceding establishment of a well-defined electron thermal distribution remain little understood. X-ray and optical probing techniques provide necessary resolution to investigate these electronic properties. Here, we will present a study of electron kinetics in warm dense gold produced by irradiating free-standing 30 nm Au foils with a 400 nm FWHM, 45 fs Ti:Sapphire laser system at SLAC National Accelerator Laboratory. The temporal evolutions of AC conductivity for 400 nm and 800 nm laser pulses are simultaneously determined with sub-100 fs resolution, providing insight into the 5 d-6 s/ p interband and 6 s / p intraband transitions respectively. Our results suggest that Auger decay and three-body recombination play important roles in electron thermalization of warm dense gold.

Laser Ablated Carbon Nanodots for Light Emission.

PubMed

Reyes, Delfino; Camacho, Marco; Camacho, Miguel; Mayorga, Miguel; Weathers, Duncan; Salamo, Greg; Wang, Zhiming; Neogi, Arup

2016-12-01

The synthesis of fluorescent carbon dots-like nanostructures (CNDs) obtained through the laser ablation of a carbon solid target in liquid environment is reported. The ablation process was induced in acetone with laser pulses of 1064, 532, and 355 nm under different irradiation times. Close-spherical amorphous CNDs with sizes between 5 and 20 nm, whose abundance strongly depends on the ablation parameters were investigated using electron microscopy and was confirmed using absorption and emission spectroscopies. The π- π* electronic transition at 3.76 eV dominates the absorption for all the CNDs species synthesized under different irradiation conditions. The light emission is most efficient due to excitation at 3.54 eV with the photoluminescence intensity centered at 3.23 eV. The light emission from the CNDs is most efficient due to ablation at 355 nm. The emission wavelength of the CNDs can be tuned from the near-UV to the green wavelength region by controlling the ablation time and modifying the ablation and excitation laser wavelength.

Analysis of laser produced plasmas of gold in the 1-7 nm region

NASA Astrophysics Data System (ADS)

Li, Bowen; Higashiguchi, Takeshi; Otsuka, Takamitsu; Yugami, Noboru; Dunne, Padraig; Kilbane, Deirdre; Sokell, Emma; O'Sullivan, Gerry

2014-04-01

Extreme ultraviolet (EUV) spectra from gold laser produced plasmas were recorded in the 1-7 nm region using two Nd:YAG lasers with pulse lengths of 150 ps and 10 ns, respectively, operating at a range of power densities. The maximum focused peak power density was 9.5 × 1013 W cm-2 for the former and 5.3 × 1012 W cm-2 for the latter. Two intense quasicontinuous intensity bands resulting from n = 4-n = 4 and n = 4-n = 5 unresolved transition arrays dominate the 4-5.5 and 1.5-3.6 nm regions of both spectra. Comparison with atomic structure calculations performed with the Cowan suite of atomic structure codes as well as consideration of previous experimental and theoretical results aided identification of the most prominent features in the spectra. For the ns spectrum, the highest ion stage that could be identified from the n = 4-n = 5 arrays was Au28+ while for the ps plasma the presence of significantly higher stages was deduced and lines due to 4d104f-4d94f2 transitions in Ag-like Au32+ give rise to the strongest observed features within the n = 4-n = 4 array while in the n = 4-n = 5 array it was possible to identify a number of previously unidentified spectral features as resulting from 4f-5g transitions in the spectra of Au XX to Au XXXIII.

Laser effect on the 248 nm KrF transition using heavy ion beam pumping

NASA Astrophysics Data System (ADS)

Adonin, A.; Jacoby, J.; Turtikov, V.; Fertman, A.; Golubev, A.; Hoffmann, D. H. H.; Ulrich, A.; Varentsov, D.; Wieser, J.

2007-07-01

In December 2005 the first successful operation of a UV excimer laser pumped with a heavy ion beam was demonstrated at GSI. It was the first experiment in which the specific power deposition was sufficient to overcome laser threshold for a UV excimer scheme. The well known KrF* excimer laser line at λ=248 nm has been chosen for this experiment, because the wavelength is short, but still in the range of usual optical diagnostic tools and the emitted light can propagate in air without attenuation. A bunch compressed U+73238 beam with a particle energy of 250 MeV/u and about 110 ns pulse duration (FWHM) was used for this experiment. Single pulses of a beam intensity up to 2.5×109 particles per bunch were focused into the laser cell along the cavity axis. Compact spectrometers, high speed UV-photodiodes and gated CCD-cameras were used for diagnostics of the spontaneous and stimulated emission. As a main result of the experiment laser effect on the 248 nm KrF* excimer laser line has been obtained and verified by temporal and spectral narrowing of the laser line as well as the threshold behaviour and exponential growth of intensity with increasing pumping power. In summary it could be shown that the pumping power of the heavy ion beam at GSI is now sufficient to pump short wavelength lasers. It is planned to extend laser experiments in near future to the VUV range of the spectrum (λ<200 nm).

Multipass pumped Nd-based thin-disk lasers: continuous-wave laser operation at 1.06 and 0.9 {mu}m with intracavity frequency doubling

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pavel, Nicolaie; Luenstedt, Kai; Petermann, Klaus

2007-12-01

The laser performances of the 1.06 {mu}m 4F3/2 --> 4I11/2 four-level transition and of the 0.9 {mu}m 4F3/2 --> I9/24 quasi-three-level transition were investigated using multipass pumped Nd-based media in thin-disk geometry. When pumping at 0.81 {mu}m into the 4F5/2 level, continuous-wave laser operation was obtained with powers in excess of 10 W at 1.06 {mu}m, in the multiwatt region at 0.91 {mu}m in Nd:YVO4 and Nd:GdVO4, and at 0.95 {mu}m in Nd:YAG. Intracavity frequency-doubled Nd:YVO4 thin-disk lasers with output powers of 6.4 W at 532 nm and of 1.6 W at 457 nm were realized at this pumping wavelength.more » The pumping at 0.88 {mu}m, which is directed into the 4F3/2 emitting level, was also employed, and Nd:YVO4 and Nd:GdVO4 thin-disk lasers with {approx}9 W output power at 1.06 {mu}m and visible laser radiation at 0.53 {mu}m with output power in excess of 4 W were realized. Frequency-doubled Nd:vanadate thin-disk lasers with deep blue emission at 0.46 {mu}m were obtained under pumping directly into the 4F3/2 emitting level.« less

Study of titania nanorod films deposited by matrix-assisted pulsed laser evaporation as a function of laser fluence

NASA Astrophysics Data System (ADS)

Caricato, A. P.; Belviso, M. R.; Catalano, M.; Cesaria, M.; Cozzoli, P. D.; Luches, A.; Manera, M. G.; Martino, M.; Rella, R.; Taurino, A.

2011-11-01

Chemically synthesized brookite titanium dioxide (TiO2) nanorods with average diameter and length dimensions of 3-4 nm and 35-50 nm, respectively, were deposited by the matrix-assisted pulsed laser evaporation technique. A toluene nanorod solution was frozen at the liquid-nitrogen temperature and irradiated with a KrF excimer laser ( λ=248 nm, τ=20 ns) at the repetition rate of 10 Hz, at different fluences (25 to 350 mJ/cm2). The deposited films were structurally characterized by high-resolution scanning and transmission electron microscopy. <100> single-crystal Si wafers and carbon-coated Cu grids were used as substrates. Structural analyses evidenced the occurrence of brookite-phase crystalline nanospheres coexisting with individually distinguishable TiO2 nanorods in the films deposited at fluences varying from 50 to 350 mJ/cm2. Nanostructured TiO2 films comprising only nanorods were deposited by lowering the laser fluence to 25 mJ/cm2. The observed shape and phase transitions of the nanorods are discussed taking into account the laser-induced heating effects, reduced melting temperature and size-dependent thermodynamic stability of nanoscale TiO2.

Application of LIF technique for the space- and time-resolved monitoring of pollutant gas decomposition in nonthermal plasma reactors

NASA Astrophysics Data System (ADS)

Mizeraczyk, Jerzy; Ohkubo, Toshikazu; Kanazawa, Seiji; Kocik, Marek

2003-10-01

Laser-induced fluorescence (LIF) technique aided by intensified CCD light signal detection and fast digital image processing is demonstrated to be a useful diagnostic method for in-situ observation of the discharge-induced plasma-chemistry processes responsible for NOx(NO + NO2) decomposition occurring in non-thermal plasma reactors. In this paper a method and results of the LIF measurement of two-dimensional distribution of the ground-state NO molecule density inside a DC positive streamer corona reactor during NO removal from a flue gas simulator [air/NO(up to 300 ppm)] are presented. Either a needle-to-plate or nozzle-to-plate electrode system, having an electrode gap of 30-50 mm was used for generating the corona discharge in the reactor. The LIF monitoring of NO molecules was carried out under the steady-state DC corona discharge condition. The laser-induced fluorescence on the transition NO X2Π(v"=0)<--A2Σ+(v'=0) at λ=226nm was chosen for monitoring ground-state NO molecules in the reactor. This transition was induced by irradiation of the NO molecules with UV laser pulses generated by a laser system consisted of a XeF excimer laser, dye laser and BBO crystal. The laser pulses from the XeF excimer laser (Lambda Physik, Complex 150, λ=351 nm) pumped the dye laser (Lambda Physik, Scanmate) with Coumarin 47 as a dye, which generated the laser beam of a wavelength turned around λ=450 nm. Then, the tuned dye laser beam pumped the BBO crystal in which the second harmonic radiation of a wavelength correspondingly tuned around λ=226 nm was generated. The 226-nm UV laser pulses of energy of 0.8-2 mJ and duration of about 20 ns were transformed into the form of the so-called laser sheet (width of 1 mm, height of 30-50 mm) which passed between the electrodes through the operating gas. The obtained results, presented in the form of images, which illustrated the two-dimensional distributions of NO molecule concentration in the non-thermal reactor, showed that the corona discharge-induced removal of NO molecules occurred not only in the vicinity of the plasma region formed by the corona discharge-induced removal of NO molecules occurred not only in the vicinity of the plasma region formed by the corona streamers and in the downstream region of the reactor but also in the upstream region of the reactor, i.e. before the flue gas simulator has entered the plasma region. This information obtained owing to the LIF technique, is important for the understanding of the plasma-chemistry processes responsible for NOx decomposition in non-thermal plasma reactors and for optimising their performance.

Laser-diode-excited blue upconversion in Tm3+/Yb3+ -codoped TeO2-Ga2O3-R2O (R=Li, Na, K) glasses.

PubMed

Zhao, Chun; Zhang, Qinyuan; Yang, Gangfeng; Jiang, Zhonghong

2008-01-01

This paper reports on intense blue upconversion in Tm(3+)/Yb(3+) codoped TeO(2)-Ga(2)O(3)-R(2)O(R=Li, Na, K) glasses upon excitation with commercial available laser diode (LD). Effects of alkali ions on the Raman spectra, thermal stability and spectroscopic properties of the tellurite-gallium glasses have also been investigated. Energy transfer and the involved upconversion mechanisms have been discussed. Intense blue upconversion emission centered at 476 nm along with a weak red emission at 650 nm has been observed upon excitation of 977 nm LD, assigned to the transitions of 1G4-->3H6, and 1G4-->3H4 and/or 3F(2,3)-->3H6 of Tm(3+), respectively. The blue upconversion intensity has a cubelike dependence on incident pump laser power, indicating a three-photon process. However, a quadratic dependence of the 476 nm upconversion intensity on the incident pump laser power has been observed when samples under excitation of 808 nm LD due to a two-photon absorption process. Enhanced upconversion luminescence have been observed with replacing K(+) for Na(+) and Li(+).

High-power Al-free active region (λ= 852nm) DFB laser diodes for atomic clocks and interferometry applications

NASA Astrophysics Data System (ADS)

Ligeret, V.; Vermersch, F.-J.; Bansropun, S.; Lecomte, M.; Calligaro, M.; Parillaud, O.; Krakowski, M.

2017-11-01

Atomic clocks will be used in the future European positioning system Galileo. Among them, the optically pumped clocks provide a better alternative with comparable accuracy for a more compact system. For these systems, diode lasers emitting at 852nm are strategic components. The laser in a conventional bench for atomic clocks presents disadvantages for spatial applications. A better approach would be to realise a system based on a distributed-feedback laser (DFB). We have developed the technological foundations of such lasers operating at 852nm. These include an Al free active region, a single spatial mode ridge waveguide and a DFB structure. The device is a separate confinement heterostructure with a GaInP large optical cavity and a single compressive strained GaInAsP quantum well. The broad area laser diodes are characterised by low internal losses (<3cm -1 ), a high internal efficiency (94%) and a low transparency current density (100A/cm2). For an AR-HR coated ridge Fabry Perot laser, we obtain a power of 230mW with M2=1.3. An optical power of 150mW was obtained at 854nm wavelength, 20°C for AR-HR coated devices. We obtain a single spatial mode emission with M2=1.21 and a SMSR over 30dB, both at 150mW. DFB Lasers at 852.12nm, corresponding to the D2 caesium transition, were then realised with a power of 40mW, 37°C for uncoated devices. The SMSR is over 30dB and the M2=1.33 at 40mW. Furthermore, the preliminary results of the linewidth obtained with a Fabry Perot interferometer give a value of less than 2MHz.

Measurement of the isotope shift of the 63 P 1 ↔53 D 1 transition of ytterbium by using a diode oscillator fiber amplified laser

NASA Astrophysics Data System (ADS)

Lee, L.; Park, H.; Ko, K.-H.; Jeong, D.-Y.

2010-08-01

We demonstrated a Diode Oscillator Fiber Amplification (DOFA) system in order to study the 63 P 1 ↔53 D 1 (1539 nm) transition line of a neutral ytterbium atom that is accessed by the stepwise excitation of the ground state. The frequency of the DOFA system was doubled by a MgO:PPLN crystal for the resonant excitation of the 61 S 0 ↔63 P 1 transition. The frequency of the second harmonic beam was stabilized to the 61 S 0 ↔63 P 1 transition of each isotope with the stability of about 2 MHz. We performed absorption spectroscopy on the 63 P 1 ↔53 D 1 (1539 nm) transition after the velocity selective excitation by the frequency-doubled beam. The isotope shifts in the 63 P 1 ↔53 D 1 (1539 nm) transition were directly measured for the first time. The relative isotope shifts from 174Yb were measured as -105.8 MHz and 109.7 MHz for 176Yb and 172Yb, respectively.

Origin of near to middle infrared luminescence and energy transfer process of Er(3+)/Yb(3+)co-doped fluorotellurite glasses under different excitations.

PubMed

Huang, Feifei; Liu, Xueqiang; Ma, Yaoyao; Kang, Shuai; Hu, Lili; Chen, Danping

2015-02-04

We report the near to middle infrared luminescence and energy transfer process of Er(3+)/Yb(3+) co-doped fluorotellurite glasses under 980, 1550 and 800 nm excitations, respectively. Using a 980 nm laser diode pump, enhanced 1.5 and 2.7 μm emissions from Er(3+):I13/2→(4)I15/2 and I11/2→(4)I13/2 transitions are observed, in which Yb(3+) ions can increase pumping efficiency and be used as energy transfer donors. Meanwhile, Yb(3+) can also be used as an acceptor and intensive upconversion luminescence of around 1000 nm is achieved from Er(3+):I11/2→(4)I15/2 and Yb(3+): F5/2→(4)F7/2 transitions using 1550 nm excitation. In addition, the luminescence properties and variation trendency by 800 nm excitation is similar to that using 1550 nm excitation. The optimum Er(3+) and Yb(3+) ion ratio is 1:1.5 and excess Yb(3+) ions decrease energy transfer efficiency under the two pumpings. These results indicate that Er(3+)/Yb(3+) co-doped fluorotellurite glasses are potential middle- infrared laser materials and may be used to increase the efficiency of the silicon solar cells.

Origin of near to middle infrared luminescence and energy transfer process of Er3+/Yb3+co-doped fluorotellurite glasses under different excitations

PubMed Central

Huang, Feifei; Liu, Xueqiang; Ma, Yaoyao; Kang, Shuai; Hu, Lili; Chen, Danping

2015-01-01

We report the near to middle infrared luminescence and energy transfer process of Er3+/Yb3+ co-doped fluorotellurite glasses under 980, 1550 and 800 nm excitations, respectively. Using a 980 nm laser diode pump, enhanced 1.5 and 2.7 μm emissions from Er3+:I13/2→4I15/2 and I11/2→4I13/2 transitions are observed, in which Yb3+ ions can increase pumping efficiency and be used as energy transfer donors. Meanwhile, Yb3+ can also be used as an acceptor and intensive upconversion luminescence of around 1000 nm is achieved from Er3+:I11/2→4I15/2 and Yb3+: F5/2→4F7/2 transitions using 1550 nm excitation. In addition, the luminescence properties and variation trendency by 800 nm excitation is similar to that using 1550 nm excitation. The optimum Er3+ and Yb3+ ion ratio is 1:1.5 and excess Yb3+ ions decrease energy transfer efficiency under the two pumpings. These results indicate that Er3+/Yb3+ co-doped fluorotellurite glasses are potential middle- infrared laser materials and may be used to increase the efficiency of the silicon solar cells. PMID:25648651

Near Infrared Laser Spectroscopy of Scandium Monobromide

NASA Astrophysics Data System (ADS)

Xia, Ye; Cheung, A. S.-C.; Liao, Zhenwu; Yang, Mei; Chan, Man-Chor

2012-06-01

High resolution laser spectrum of scandium monobromide (ScBr) between 787 and 845 nm has been investigated using the technique of laser vaporization/reaction with free jet expansion and laser induced fluorescence spectroscopy. ScBr was produced by reacting laser vaporized Sc atoms with ethyl bromide (C2H5Br). Spectra of six vibrational bands of both Sc79Br and Sc81Br isotopomers of the C1 Σ+ - X1 Σ+ transition and seven vibrational bands of the e3 Δ - a3 Δ transition were obtained and analyzed. Least-squares fit of the measured line positions for the singlet transitions yielded accurate molecular constants for the v = 0 - 3 levels of the C1 Σ+ state and the v = 0 - 2 levels of the X1 Σ+ state. Similar least-squares fit for the triplet transitions yielded molecular constants for the v = 0 - 2 levels of both e3 Δ and a3 Δ states. The equilibrium bond length, r_0, of the a3 Δ state has been determined to be 2.4789 Å. Financial support from the Research Grants Council of the Hong Kong Special Administrative Region, China (Project No. HKU 701008P) is gratefully acknowledged

Atomic processes and equation of state of high Z plasmas for EUV sources and their effects on the spatial and temporal evolution of the plasmas

NASA Astrophysics Data System (ADS)

Sasaki, Akira; Sunahara, Atushi; Furukawa, Hiroyuki; Nishihara, Katsunobu; Nishikawa, Takeshi; Koike, Fumihiro

2016-03-01

Laser-produced plasma (LPP) extreme ultraviolet (EUV) light sources have been intensively investigated due to potential application to next-generation semiconductor technology. Current studies focus on the atomic processes and hydrodynamics of plasmas to develop shorter wavelength sources at λ = 6.x nm as well as to improve the conversion efficiency (CE) of λ = 13.5 nm sources. This paper examines the atomic processes of mid-z elements, which are potential candidates for λ = 6.x nm source using n=3-3 transitions. Furthermore, a method to calculate the hydrodynamics of the plasmas in terms of the initial interaction between a relatively weak prepulse laser is presented.

Short wavelength (visible) GaAs quantum well lasers grown by molecular beam epitaxy

DOE Office of Scientific and Technical Information (OSTI.GOV)

Woodbridge, K.; Blood, P.; Fletcher, E.D.

1984-07-01

GaAs-AlGaAs multiple quantum well (MQW) injection lasers with well widths from 55 to 13 A have been grown by molecular beam epitaxy and operated at room temperature, showing emission at wavelengths down to 704 nm, the shortest reported for a MQW injection laser with GaAs wells. In a device with 25-A wells some evidence of coupling was apparent when barrier widths were reduced to 40 A. For devices with 80-A barriers there is a difference of about 20 nm between the calculated n = 1 (e--hh) transition wavelength and the lasing wavelength, whereas the calculation agrees with photovoltage absorption measurementsmore » on the same structures.« less

Optical absorbances of Gd3Ga5O12 single crystals under shock compression to 211 GPa

NASA Astrophysics Data System (ADS)

Liu, Q. C.; Zhou, X. M.; Luo, S. N.

2017-04-01

Shock-induced opacity in Gd3Ga5O12 (GGG) single crystals is investigated by transmission/emission measurements at 16 wavelengths (400-800 nm), as well as complementary particle velocity measurements at 1550 nm, in the pressure range of 47-211 GPa. Optical transmission spectra through the shocked samples are measured with a in-situ, shock-generated light source, and the resultant extinction coefficients of different wavelengths and shock pressures obtained. As shock strength increases, the optical opacity of the shocked GGG increases and peaks at 75 GPa (the transparent-opaque transition), drops at 75-100 GPa (the opaque-transparent transition), and then increases again. The transparency recovery coincides with a solid-solid phase transition. The microstructure changes associated with the solid-solid phase transition and plastic deformation most likely cause the loss and recovery of transparency. GGG can be useful as a high pressure window for laser velocimetry (1550 nm) or optical pyrometry (400-800 nm) in the ranges of 100-140 GPa and 80-120 GPa, respectively.

Thickness driven spin reorientation transition of epitaxial LaCrO3 films

NASA Astrophysics Data System (ADS)

Park, Junho; Kim, Dong-Hwan; Lee, Doopyo; Ko, Kyung-Tae; Hyun Song, Jong; Kim, Jae-Young; Koo, Tae-Yeong; Lee, Seung Ran; Park, Jae-Hoon

2018-03-01

We grew fully strained epitaxial LaCrO3 (LCO) films on SrTiO3(001) under layer-by-layer control up to the film thickness of t = 130 nm using a pulsed laser deposition method. The spin axis of the antiferromagnetic LCO film was systematically examined as a function of t by using Cr L2,3-edge x-ray magnetic linear dichroism (XMLD). The XMLD results manifest a spin reorientation transition (SRT) across a transition thickness of tT ˜ 60 nm. This SRT is well explained in terms of two competing magnetic anisotropy energies of the surface/interface (KS) and the LCO film itself (KV).

Frequency measurement of the 5 S{1}/{2}(F = 3)-5 D{5}/{2}(F = 5) two-photon transition in rubidium

NASA Astrophysics Data System (ADS)

Touahri, D.; Acef, O.; Clairon, A.; Zondy, J.-J.; Felder, R.; Hilico, L.; de Beauvoir, B.; Biraben, F.; Nez, F.

1997-02-01

We have measured the frequencies of three diode lasers stabilized on the 5 S{1}/{2}(F = 3)-5 D{5}/{2}(F = 5) two-photon transition in rubidium at λ = 778.1 nm, with an uncertainty of 1 kHz, using BNM-LPTF frequency synthesis chain starting from a {CO 2}/{OsO 4} reference laser at 10.3 μm. We show that this frequency chain is able to reach the 10 -13 resolution level. After a discussion of the systematic effects that may shift the resonance, the transition frequency is found to be ν = 385 285 142 378.280 ± 2 kHz.

Controllable red, green, blue (RGB) and bright white upconversion luminescence of Lu2O3:Yb3+/Er3+/Tm3+ nanocrystals through single laser excitation at 980 nm.

PubMed

Yang, Jun; Zhang, Cuimiao; Peng, Chong; Li, Chunxia; Wang, Lili; Chai, Ruitao; Lin, Jun

2009-01-01

Light fantastic! Lu(2)O(3):Yb(3+)/Er(3+)/Tm(3+) nanocrystals with controllable red, green, blue (RGB) and bright white upconversion luminescence by a single laser excitation of 980 nm have been successfully synthesized (see picture). Due to abundant UC PL colors, it can potentially be used as fluorophores in the field of color displays, back light, UC lasers, photonics, and biomedicine.Lu(2)O(3):Yb(3+)/Er(3+)/Tm(3+) nanocrystals have been successfully synthesized by a solvothermal process followed by a subsequent heat treatment at 800 degrees C. Powder X-ray diffraction, transmission electron microscopy, upconversion photoluminescence spectra, and kinetic decay were used to characterize the samples. Under single-wavelength diode laser excitation of 980 nm, the bright blue emissions of Lu(2)O(3):Yb(3+), Tm(3+) nanocrystals near 477 and 490 nm were observed due to the (1)G(4)-->(3)H(6) transition of Tm(3+). The bright green UC emissions of Lu(2)O(3):Er(3+) nanocrystals appeared near 540 and 565 nm were observed and assigned to the (2)H(11/2)-->(4)I(15/2) and (4)S(3/2)-->(4)I(15/2) transitions, respectively, of Er(3+). The ratio of the intensity of green luminescence to that of red luminescence decreases with an increase of concentration of Yb(3+) in Lu(2)O(3):Er(3+) nanocrystals. In sufficient quantities of Yb(3+) with resprct to Er(3+), the bright red UC emission of Lu(2)O(3):Yb(3+)/Er(3+) centered at 662 nm was predominant, due to the (4)F(9/2)-->(4)I(15/2) transition of Er(3+). Based on the generation of red, green, and blue emissions in the different doped Lu(2)O(3):RE(3+) nanocrystals, it is possible to produce the luminescence with a wide spectrum of colors, including white, by the appropriate doping of Yb(3+), Tm(3+), and Er(3+) in the present Lu(2)O(3) nanocrystals. Namely, Lu(2)O(3):3 %Yb(3+)/0.2 %Tm(3+)/0.4 %Er(3+) nanocrystals show suitable intensities of blue, green, and red (RGB) emission, resulting in the production of perfect and bright white light with CIE-x=0.3456 and CIE-y=0.3179, which is very close to the standard equal energy white light illuminate (x=0.33, y=0.33). Because of abundant luminescent colors from RGB to white in Lu(2)O(3):Yb(3+)/Er(3+)/Tm(3+) nanocrystals under 980 nm laser diode (LD) excitation, they can potentially be used as fluorophores in the field of color displays, back light, UC lasers, photonics, and biomedicine.

Laser induced fluorescence in Ar and He plasmas with a tunable diode laser

NASA Astrophysics Data System (ADS)

Boivin, R. F.; Scime, E. E.

2003-10-01

A diode laser based laser induced fluorescence (LIF) diagnostic that uses an inexpensive diode laser system is described. This LIF diagnostic has been developed on the hot helicon experiment (HELIX) plasma device. The same diode laser is used to alternatively pump Ar II and He I transitions to obtain argon ion and atomic helium temperatures, respectively. The 1.5 MHz bandwidth diode laser has a Littrow external cavity with a mode-hop free tuning range up to 14 GHz (≈0.021 nm) and a total power output of about 12 mW. Wavelength scanning is achieved by varying the voltage on a piezoelectric controlled grating located within the laser cavity. The fluorescence radiation is monitored with a photomultiplier detector. A narrow band interference filter is used to eliminate all but the plasma radiation in the immediate vicinity of the fluorescence wavelength. Lock-in amplification is used to isolate the fluorescence signal from noise and electron-impact induced radiation. For the Ar ion, the laser tuned at 668.43 nm is used to pump the 3d 4F7/2 Ar II metastable level to the 4p 4D5/2 level. The 442.60 nm fluorescence radiation between the 4p 4D5/2 and the 4s 4P3/2 levels is captured by the photomultiplier tube. For atomic He, the laser is tuned at 667.82 nm to pump a fraction of the electron population from the 21P state to the 31D upper level. Although the 21P level is not a metastable, the close proximity of 21S metastable makes this new He I LIF scheme possible. In this scheme, a fraction of the laser-excited electrons undergo collisional excitation transfer from the 31D to the 31P level. In turn, the 31P state decays to the metastable 21S by emitting 501.57 nm fluorescence photons.

Development of a Discharge Pumped 13 nm Laser for Metrology of Projection Lithography Optics at the Manufacture-Site

DTIC Science & Technology

2003-09-14

nm @2,6,9#. In the particular case of Ar discharges the gain-length product for the 3p 1S0-3s 1P1 transition of Ne-like Ar at 46.9 nm has exceeded...The addition of the Al filter decreases the transmissivity in this window by a factor that increases from about 63 at 4.5 nm to about 6003 at 10 nm... factors including the smaller current and pinch radius, together with very good initial plasma symmetry and relatively short time duration of4-7 GONZALEZ

A simplified scheme for generating narrow-band mid-ultraviolet laser radiation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Almog, G.; Ludwig-Maximilians-Universität, Geschwister-Scholl-Platz 1, 80539 München; Scholz, M., E-mail: Matthias.Scholz@toptica.com

2015-03-15

We report on the development and characterization of continuous, narrow-band, and tunable laser systems that use direct second-harmonic generation from blue and green diode lasers with an output power level of up to 11.1 mW in the mid-ultraviolet. One of our laser systems was tuned to the mercury 6{sup 1}S{sub 0} → 6{sup 3}P{sub 1} intercombination line at 253.7 nm. We could perform Doppler-free saturation spectroscopy on this line and were able to lock our laser to the transition frequency on long time scales.

LASER RADIATION CHARACTERISTICS (BRIEF COMMUNICATIONS): Conversion of KrCl and XeCl laser radiation to the visible spectral range by stimulated Raman scattering in lead vapor

NASA Astrophysics Data System (ADS)

Evtushenko, Gennadii S.; Mel'chenko, S. V.; Panchenko, Aleksei N.; Tarasenko, Viktor F.

1990-04-01

Conversion of KrCl and XeCl laser radiation by stimulated Raman scattering was achieved in lead vapor. The KrCl laser radiation was converted into three lines in the visible region at λ = 406, 590, and 723 nm by transitions from both the ground and first excited levels of the lead atom. The conversion efficiency of XeCl laser radiation of low spatial coherence was found to be limited by the activation of a competing nonlinear process.

Compact Optical Atomic Clock Based on a Two-Photon Transition in Rubidium

NASA Astrophysics Data System (ADS)

Martin, Kyle W.; Phelps, Gretchen; Lemke, Nathan D.; Bigelow, Matthew S.; Stuhl, Benjamin; Wojcik, Michael; Holt, Michael; Coddington, Ian; Bishop, Michael W.; Burke, John H.

2018-01-01

Extralaboratory atomic clocks are necessary for a wide array of applications (e.g., satellite-based navigation and communication). Building upon existing vapor-cell and laser technologies, we describe an optical atomic clock, designed around a simple and manufacturable architecture, that utilizes the 778-nm two-photon transition in rubidium and yields fractional-frequency instabilities of 4 ×10-13/√{τ (s ) } for τ from 1 to 10 000 s. We present a complete stability budget for this system and explore the required conditions under which a fractional-frequency instability of 1 ×10-15 can be maintained on long time scales. We provide a precise characterization of the leading sensitivities to external processes, including magnetic fields and fluctuations of the vapor-cell temperature and 778-nm laser power. The system is constructed primarily from commercially available components, an attractive feature from the standpoint of the commercialization and deployment of optical frequency standards.

Innovative scheme for high-repetition-rate imaging of CN radical.

PubMed

Satija, Aman; Ruesch, Morgan D; Powell, Michael S; Son, Steven F; Lucht, Robert P

2018-02-01

We have employed, to the best of our knowledge, a novel excitation scheme to perform the first high-repetition-rate planar laser-induced fluorescence (PLIF) measurements of a CN radical in combustion. The third harmonic of a Nd:YVO 4 laser at 355 nm due to its relatively large linewidth overlaps with several R branch transitions in a CN ground electronic state. Therefore, the 355 nm beam was employed to directly excite the CN transitions with good efficiency. The CN measurements were performed in premixed CH 4 -N 2 O flames with varying equivalence ratios. A detailed characterization of the high-speed CN PLIF imaging system is presented via its ability to capture statistical and dynamical information in these premixed flames. Single-shot CN PLIF images obtained over a HMX pellet undergoing self-supported deflagration are presented as an example of the imaging system being applied towards characterizing the flame structure of energetic materials.

Direct spectral analysis and determination of high content of carcinogenic bromine in bread using UV pulsed laser induced breakdown spectroscopy.

PubMed

Mehder, A O; Gondal, Mohammed A; Dastageer, Mohamed A; Habibullah, Yusuf B; Iqbal, Mohammed A; Oloore, Luqman E; Gondal, Bilal

2016-01-01

Laser induced breakdown spectroscopy (LIBS) was applied for the detection of carcinogenic elements like bromine in four representative brands of loaf bread samples and the measured bromine concentrations were 352, 157, 451, and 311 ppm, using Br I (827.2 nm) atomic transition line as the finger print atomic transition. Our LIBS system is equipped with a pulsed laser of wavelength 266 nm with energy 25 mJ pulse(-1), 8 ns pulse duration, 20 Hz repetition rate, and a gated ICCD camera. The LIBS system was calibrated with the standards of known concentrations in the sample (bread) matrix and such plot is linear in 20-500 ppm range. The capability of our system in terms of limit of detection and relative accuracy with respect to the standard inductively coupled plasma mass spectrometry (ICPMS) technique was evaluated and these values were 5.09 ppm and 0.01-0.05, respectively, which ensures the applicability of our system for Br trace level detection, and LIBS results are in excellent agreement with that of ICPMS results.

Trapping, retention and laser cooling of Th3+ ions in a multisection linear quadrupole trap

NASA Astrophysics Data System (ADS)

Borisyuk, P. V.; Vasil'ev, O. S.; Derevyashkin, S. P.; Kolachevsky, N. N.; Lebedinskii, Yu. Yu.; Poteshin, S. S.; Sysoev, A. A.; Tkalya, E. V.; Tregubov, D. O.; Troyan, V. I.; Khabarova, K. Yu.; Yudin, V. I.; Yakovlev, V. P.

2017-06-01

A multisection linear quadrupole trap for Th3+ ions is described. Multiply charged ions are obtained by the laser ablation method. The possibility of trapping and retention of ˜103 ions is demonstrated in macroscopic time scales of ˜30 s. Specific features of cooling Th3+ ions on the electron transitions with wavelengths of 1088, 690 and 984 nm in Th3+ ion are discussed; a principal scheme of a setup for laser cooling is presented.

Radioluminescence and photoluminescence of Th:CaF2 crystals

PubMed Central

Stellmer, Simon; Schreitl, Matthias; Schumm, Thorsten

2015-01-01

We study thorium-doped CaF2 crystals as a possible platform for optical spectroscopy of the 229Th nuclear isomer transition. We anticipate two major sources of background signal that might cover the nuclear spectroscopy signal: VUV-photoluminescence, caused by the probe light, and radioluminescence, caused by the radioactive decay of 229Th and its daughters. We find a rich photoluminescence spectrum at wavelengths above 260 nm, and radioluminescence emission above 220 nm. This is very promising, as fluorescence originating from the isomer transition, predicted at a wavelength shorter than 200 nm, could be filtered spectrally from the crystal luminescence. Furthermore, we investigate the temperature-dependent decay time of the luminescence, as well as thermoluminescence properties. Our findings allow for an immediate optimization of spectroscopy protocols for both the initial search for the nuclear transition using synchrotron radiation, as well as future optical clock operation with narrow-linewidth lasers. PMID:26502749

A new ~1 μm laser crystal Nd:Gd2SrAl2O7: growth, thermal, spectral and lasing properties

NASA Astrophysics Data System (ADS)

Yuan, Feifei; Liao, Wenbin; Huang, Yisheng; Zhang, Lizhen; Sun, Shijia; Wang, Yeqing; Lin, Zhoubin; Wang, Guofu; Zhang, Ge

2018-03-01

Nd:Gd2SrAl2O7 crystals were grown by the Czochralski technique; thermal, spectral and laser properties were investigated in detail. The average thermal expansion coefficients along a- and c-axis are 12.6  ×  10-6 K-1 and 14.9  ×  10-6 K-1, respectively. At room temperature, the thermal conductivities are 4.98 and 5.24 W (m-1 * K-1) along the a- and c-axis, respectively. The absorption cross sections at ~808 nm are 13.7  ×  10-20 cm2 with a FWHM of 3.3 nm for π-polarization and 11.84  ×  10-20 cm2 with a FWHM of 3.4 nm for σ-polarization. The emission cross sections at ~1080 nm are 15  ×  10-20 cm2 and 12.7  ×  10-20 cm2 with a FWHM of about 5.1 nm and 12.5 nm for π- and σ-polarization, respectively. The fluorescence lifetime for the 4F3/2  →  4I11/2 transition was fitted to be 118 µs. Pumped by a fiber-coupled 808 nm laser diode, the maximum 1.55 W continuous-wave laser output at ~1.08 µm was achieved with a slope efficiency of 30.5%. All the results show that Nd:Gd2SrAl2O7 crystal is a promising laser material.

Room-temperature subnanosecond waveguide lasers in Nd:YVO4 Q-switched by phase-change VO2: A comparison with 2D materials

NASA Astrophysics Data System (ADS)

Nie, Weijie; Li, Rang; Cheng, Chen; Chen, Yanxue; Lu, Qingming; Romero, Carolina; Vázquez de Aldana, Javier R.; Hao, Xiaotao; Chen, Feng

2017-04-01

We report on room-temperature subnanosecond waveguide laser operation at 1064 nm in a Nd:YVO4 crystal waveguide through Q-switching of phase-change nanomaterial vanadium dioxide (VO2). The unique feature of VO2 nanomaterial from the insulating to metallic phases offers low-saturation-intensity nonlinear absorptions of light for subnanosecond pulse generation. The low-loss waveguide is fabricated by using the femtosecond laser writing with depressed cladding geometry. Under optical pump at 808 nm, efficient pulsed laser has been achieved in the Nd:YVO4 waveguide, reaching minimum pulse duration of 690 ps and maximum output average power of 66.7 mW. To compare the Q-switched laser performances by VO2 saturable absorber with those based on two-dimensional materials, the 1064-nm laser pulses have been realized in the same waveguide platform with either graphene or transition metal dichalcogenide (in this work, WS2) coated mirror. The results on 2D material Q-switched waveguide lasers have shown that the shortest pulses are with 22-ns duration, whilst the maximum output average powers reach ~161.9 mW. This work shows the obvious difference on the lasing properties based on phase-change material and 2D materials, and suggests potential applications of VO2 as low-cost saturable absorber for subnanosecond laser generation.

Room-temperature subnanosecond waveguide lasers in Nd:YVO4 Q-switched by phase-change VO2: A comparison with 2D materials.

PubMed

Nie, Weijie; Li, Rang; Cheng, Chen; Chen, Yanxue; Lu, Qingming; Romero, Carolina; Vázquez de Aldana, Javier R; Hao, Xiaotao; Chen, Feng

2017-04-06

We report on room-temperature subnanosecond waveguide laser operation at 1064 nm in a Nd:YVO 4 crystal waveguide through Q-switching of phase-change nanomaterial vanadium dioxide (VO 2 ). The unique feature of VO 2 nanomaterial from the insulating to metallic phases offers low-saturation-intensity nonlinear absorptions of light for subnanosecond pulse generation. The low-loss waveguide is fabricated by using the femtosecond laser writing with depressed cladding geometry. Under optical pump at 808 nm, efficient pulsed laser has been achieved in the Nd:YVO 4 waveguide, reaching minimum pulse duration of 690 ps and maximum output average power of 66.7 mW. To compare the Q-switched laser performances by VO 2 saturable absorber with those based on two-dimensional materials, the 1064-nm laser pulses have been realized in the same waveguide platform with either graphene or transition metal dichalcogenide (in this work, WS 2 ) coated mirror. The results on 2D material Q-switched waveguide lasers have shown that the shortest pulses are with 22-ns duration, whilst the maximum output average powers reach ~161.9 mW. This work shows the obvious difference on the lasing properties based on phase-change material and 2D materials, and suggests potential applications of VO 2 as low-cost saturable absorber for subnanosecond laser generation.

Ionization cross section, pressure shift and isotope shift measurements of osmium

NASA Astrophysics Data System (ADS)

Hirayama, Yoshikazu; Mukai, Momo; Watanabe, Yutaka; Oyaizu, Michihiro; Ahmed, Murad; Kakiguchi, Yutaka; Kimura, Sota; Miyatake, Hiroari; Schury, Peter; Wada, Michiharu; Jeong, Sun-Chan

2017-11-01

In-gas-cell laser resonance ionization spectroscopy of neutral osmium atoms was performed with the use of a two-color two-step laser resonance ionization technique. Saturation curves for the ionization scheme were measured, and the ionization cross section was experimentally determined by solving the rate equations for the ground, intermediate and ionization continuum populations. The pressure shift and pressure broadening in the resonance spectra of the excitation transition were measured. The electronic factor {F}247 for the transition {λ }1=247.7583 nm to the intermediate state was deduced from the measured isotope shifts of stable {}{188,189,{190,192}}Os isotopes. The efficient ionization scheme, pressure shift, nuclear isotope shift and {F}247 are expected to be useful for applications of laser ion sources to unstable nuclei and for nuclear spectroscopy based on laser ionization techniques.

Photoionization and trans-to-cis isomerization of β-cyclodextrin-encapsulated azobenzene induced by two-color two-laser-pulse excitation.

PubMed

Takeshita, Tatsuya; Hara, Michihiro

2018-03-15

Azobenzene (1) and the complex resulting from the incorporation of 1 with cyclodextrin (1/CD) are attractive for light-driven applications such as micromachining and chemical biology tools. The highly sensitive photoresponse of 1 is crucial for light-driven applications containing both 1 and 1/CD to reach their full potential. In this study, we investigated the photoionization and trans-to-cis isomerization of 1/CD induced by one- and two-color two-laser pulse excitation. Photoionization of 1/CD, which was induced by stepwise two-photon absorption, was observed using laser pulse excitation at 266nm. Additionally, simultaneous irradiation with 266 and 532nm laser pulses increased the trans-to-cis isomerization yield (Υ t→c ) by 27%. It was concluded that the increase in Υ t→c was caused by the occurrence of trans-to-cis isomerization in the higher-energy singlet state (S n ), which was reached by S 1 →S n transition induced by laser pulse excitation at 532nm. The results of this study are potentially applicable in light-driven applications such as micromachining and chemical biology tools. Copyright © 2018 Elsevier B.V. All rights reserved.

Implications of the temperature dependence of Nd:YAG spectroscopic values for low temperature laser operation at 946 nm

NASA Astrophysics Data System (ADS)

Yoon, S. J.; Mackenzie, J. I.

2014-05-01

We present our measurements of the key spectroscopic properties over the temperature range of 77 K to 450 K for Nd3+ ions doped in Y3Al5O12 (YAG). From room to liquid nitrogen temperature (LNT), the peak absorption cross section around 808 nm increased by almost 3 times, in conjunction the bandwidth of this absorption line reduced by the same factor. At LNT the peak of the absorption line was blue shifted by 0.25 nm with respect to that at 300 K. The fluorescence spectrum between 850 nm - 1450 nm was measured, from which the emission cross sections for the three main transitions were calculated. One note of particular interest for the dominant emission wavelengths around 1064nm and 1061nm (4F3/2 --> 4I11/2) was the switch in their relative strength below 170K, and at LNT the 1061 nm line has almost twice the cross section as at 1064nm.. The fluorescence and lifetime of the upper laser level (4F3/2) was measured and the effective emission cross section determined by the Fuchtbauer-Ladenburg (F-L) method. The effective emission cross section for 946 nm (R1 --> Z5) increased by more than two times over the 300 K to 77 K range. A numerical fit for the temperature dependent emission cross section at 946 nm and 1064 nm and also calculated absorption coefficient at 808 nm pump diode laser have also obtained from the measured spectroscopic data.

Iodine-stabilized single-frequency green InGaN diode laser.

PubMed

Chen, Yi-Hsi; Lin, Wei-Chen; Shy, Jow-Tsong; Chui, Hsiang-Chen

2018-01-01

A 520-nm InGaN diode laser can emit a milliwatt-level, single-frequency laser beam when the applied current slightly exceeds the lasing threshold. The laser frequency was less sensitive to diode temperature and could be finely tuned by adjusting the applied current. Laser frequency was stabilized onto a hyperfine component in an iodine transition through the saturated absorption spectroscopy. The uncertainty of frequency stabilization was approximately 8×10 -9 at a 10-s integration time. This compact laser system can replace the conventional green diode-pumped solid-state laser and applied as a frequency reference. A single longitudinal mode operational region with diode temperature, current, and output power was investigated.

Tungsten diselenide for mode-locked erbium-doped fiber lasers with short pulse duration

NASA Astrophysics Data System (ADS)

Liu, Wenjun; Liu, Mengli; OuYang, Yuyi; Hou, Huanran; Ma, Guoli; Lei, Ming; Wei, Zhiyi

2018-04-01

In this paper, a WSe2 film prepared by chemical vapor deposition (CVD) is transferred onto a tapered fiber, and a WSe2 saturable absorber (SA) is fabricated. In order to measure the third-order optical nonlinearity of the WSe2, the Z-scan technique is applied. The modulation depth of the WSe2 SA is measured as being 21.89%. Taking advantage of the remarkable nonlinear absorption characteristic of the WSe2 SA, a mode-locked erbium-doped fiber laser is demonstrated at 1557.4 nm with a bandwidth of 25.8 nm and signal to noise ratio of 96 dB. To the best of our knowledge, the pulse duration of 163.5 fs is confirmed to be the shortest compared with previous mode-locked fiber lasers based on transition-metal dichalcogenides SAs. These results indicate that WSe2 is a powerful competitor in the application of ultrashort pulse lasers.

Tapered fluorotellurite microstructured fibers for broadband supercontinuum generation.

PubMed

Wang, Fang; Wang, Kangkang; Yao, Chuanfei; Jia, Zhixu; Wang, Shunbin; Wu, Changfeng; Qin, Guanshi; Ohishi, Yasutake; Qin, Weiping

2016-02-01

Fluorotellurite microstructured fibers (MFs) based on TeO2-BaF2-Y2O3 glasses are fabricated by using a rod-in-tube method. Tapered fluorotellurite MFs with varied transition region lengths are prepared by employing an elongation machine. By using a tapered fluorotellurite MF with a transition region length of ∼3.3  cm as the nonlinear medium and a 1560 nm femtosecond fiber laser as the pump source, broadband supercontinuum generation covering from 470 to 2770 nm is obtained. The effects of the transition region length of the tapered fluorotellurite MF on supercontinuum generation are also investigated. Our results show that tapered fluorotellurite MFs are promising nonlinear media for generating broadband supercontinuum light expanding from visible to mid-infrared spectral region.

Absolute frequency of cesium 6S-8S 822 nm two-photon transition by a high-resolution scheme.

PubMed

Wu, Chien-Ming; Liu, Tze-Wei; Wu, Ming-Hsuan; Lee, Ray-Kuang; Cheng, Wang-Yau

2013-08-15

We present an alternative scheme for determining the frequencies of cesium (Cs) atom 6S-8S Doppler-free transitions. With the use of a single electro-optical crystal, we simultaneously narrow the laser linewidth, lock the laser frequency, and resolve a narrow spectrum point by point. The error budget for this scheme is presented, and we prove that the transition frequency obtained from the Cs cell at room temperature and with one-layer μ-metal shielding is already very near that for the condition of zero collision and zero magnetic field. We point out that a sophisticated linewidth measurement could be a good guidance for choosing a suitable Cs cell for better frequency accuracy.

Thermal Characterization, Crystal Field Analysis and In-Band Pumped Laser Performance of Er Doped NaY(WO4)2 Disordered Laser Crystals

PubMed Central

Serrano, María Dolores; Cascales, Concepción; Han, Xiumei; Zaldo, Carlos; Jezowski, Andrzej; Stachowiak, Piotr; Ter-Gabrielyan, Nikolay; Fromzel, Viktor; Dubinskii, Mark

2013-01-01

Undoped and Er-doped NaY(WO4)2 disordered single crystals have been grown by the Czochralski technique. The specific heat and thermal conductivity (κ) of these crystals have been characterized from T = 4 K to 700 K and 360 K, respectively. It is shown that κ exhibits anisotropy characteristic of single crystals as well as a κ(T) behavior observed in glasses, with a saturation mean free phonon path of 3.6 Å and 4.5 Å for propagation along a and c crystal axes, respectively. The relative energy positions and irreducible representations of Stark Er3+ levels up to 4G7/2 multiplet have been determined by the combination of experimental low (<10 K) temperature optical absorption and photoluminescence measurements and simulations with a single-electron Hamiltonian including both free-ion and crystal field interactions. Absorption, emission and gain cross sections of the 4I13/2↔4I15/2 laser related transition have been determined at 77 K. The 4I13/2 Er3+ lifetime (τ) was measured in the temperature range of 77–300 K, and was found to change from τ (77K) ≈ 4.5 ms to τ (300K) ≈ 3.5 ms. Laser operation is demonstrated at 77 K and 300 K by resonantly pumping the 4I13/2 multiplet at λ≈1500 nm with a broadband (FWHM≈20 nm) diode laser source perfectly matching the 77 K crystal 4I15/2 → 4I13/2 absorption profile. At 77 K as much as 5.5 W of output power were obtained in π-polarized configuration with a slope efficiency versus absorbed pump power of 57%, the free running laser wavelength in air was λ≈1611 nm with the laser output bandwidth of 3.5 nm. The laser emission was tunable over 30.7 nm, from 1590.7 nm to 1621.4 nm, for the same π-polarized configuration. PMID:23555664

Corneal thermal damage threshold dependence on the exposure duration for near-infrared laser radiation at 1319 nm

NASA Astrophysics Data System (ADS)

Wang, Jiarui; Jiao, Luguang; Chen, Hongxia; Yang, Zaifu; Hu, Xiangjun

2016-01-01

The corneal damage effects induced by 1319-nm transitional near-infrared laser have been investigated for years. However, the damage threshold dependence on exposure duration has not been revealed. The in vivo corneal damage thresholds (ED50s) were determined in New Zealand rabbits for 1319-nm laser radiation for exposure durations from 75 ms to 10 s. An additional corneal ED50 was determined at 1338 nm for a 5-ms exposure. The incident corneal irradiance diameter was fixed at 2 mm for all exposure conditions to avoid the influence of spot size on threshold. The ED50s given in terms of the corneal radiant exposure for exposure durations of 5 ms, 75 ms, 0.35 s, 2 s, and 10 s were 39.4, 51.5, 87.2, 156.3, and 311.1 J/cm2, respectively. The 39.4 J/cm2 was derived from the ED50 for 1338 nm (27.0 J/cm2). The ED50s for exposure durations of 75 ms to 10 s were correlated by a power law equation, ED50=128.9t0.36 in J/cm2, where t was the input in the unit of second, with correlation coefficient (R) of 0.997. Enough safe margins existed between the ED50s and the maximum permitted exposures from current laser safety standard.

Searching for U-235m produced by Nuclear Excitation by Electronic Transition

NASA Astrophysics Data System (ADS)

Chodash, Perry; Norman, Eric; Burke, Jason; Wilks, Scott; Casperson, Robert

2014-09-01

Nuclear excitation by electronic transition (NEET) is a rare nuclear excitation that is predicted to occur in numerous isotopes, including U-235. When a nuclear transition matches the energy and the multipolarity of an electronic transition, there is a possibility that NEET will occur. If NEET were to occur in U-235, the nucleus would be excited to its 1/2 + isomeric state that subsequently decays by internal conversion with a decay energy of 77 eV and a half-life of 26 minutes. Theory predicts that NEET can occur in partially ionized uranium plasma with a charge state of 23 +. A pulsed Nd:YAG laser operating at 1064 nm with a pulse energy of 780 mJ and a pulse width of 9 ns was used to generate the uranium plasma. The laser was focused on small samples of both depleted uranium and highly enriched uranium. The plasma conditions created by the intense laser pulse were varied by changing the spot size of the laser on the target. The resulting plasma was collected on a plate and the internal conversion electrons were focused onto a microchannel plate detector by a series of electrostatic lenses. First results will be presented. Nuclear excitation by electronic transition (NEET) is a rare nuclear excitation that is predicted to occur in numerous isotopes, including U-235. When a nuclear transition matches the energy and the multipolarity of an electronic transition, there is a possibility that NEET will occur. If NEET were to occur in U-235, the nucleus would be excited to its 1/2 + isomeric state that subsequently decays by internal conversion with a decay energy of 77 eV and a half-life of 26 minutes. Theory predicts that NEET can occur in partially ionized uranium plasma with a charge state of 23 +. A pulsed Nd:YAG laser operating at 1064 nm with a pulse energy of 780 mJ and a pulse width of 9 ns was used to generate the uranium plasma. The laser was focused on small samples of both depleted uranium and highly enriched uranium. The plasma conditions created by the intense laser pulse were varied by changing the spot size of the laser on the target. The resulting plasma was collected on a plate and the internal conversion electrons were focused onto a microchannel plate detector by a series of electrostatic lenses. First results will be presented. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The U.S. DHS, UC Berkeley, the NNIS fellowship and the NSSC further supported this work.

Development of compact excimer lasers for remote sensing

NASA Technical Reports Server (NTRS)

Laudenslager, J. B.; Mcdermid, I. S.; Pacala, T. J.

1983-01-01

The capabilities of excimer lasers for remote sensing applications are illustrated in a discussion of the development of a compact tunable XeCl excimer laser for the detection of atmospheric OH radicals. Following a brief review of the operating principles and advantages of excimer lasers, measurements of the wavelength dependence of the net small signal gain coefficient of a discharge excited XeCl laser are presented which demonstrate the overlap of several absorption lines of the A-X(0,0) transition of OH near 308 nm with the wavelengths of the XeCl laser. A range of continuous narrow bandwidth tunability of from 307.6 to 308.4 nm with only a 30 percent variation in output is reported for an XeCl laser used as a double-pass amplifier for a frequency-doubled dye laser, and measurements demonstrating the detection of laser-induced fluorescence from OH in a methane-oxygen flame are also noted. The design of an oscillator-amplifier excimer system comprising a corona-preionized, transverse-discharge oscillator and amplifier is then presented. Output energies of 12-15 mJ have been achieved in the regions where injection locking was established, with energies of 8-10 mJ elsewhere.

Temperature measurement in a compressible flow field using laser-induced iodine fluorescence

NASA Technical Reports Server (NTRS)

Fletcher, D. G.; Mcdaniel, J. C.

1987-01-01

The thermometric capability of a two-line fluorescence technique using iodine seed molecules in air is investigated analytically and verified experimentally in a known steady compressible flow field. Temperatures ranging from 165 to 295 K were measured in the flowfield using two iodine transitions accessed with a 30-GHz dye-laser scan near 543 nm. The effect of pressure broadening on temperature measurement is evaluated.

Quantum Electronics in the UK. A National-Survey Conference.

DTIC Science & Technology

1985-10-30

flashlamp pumped chromium action, including transitions in dopants doped gadolinium /scandium/gallium garnet which have not previously shown laser lasers...frac- factors that limit performance. They ture. The Southampton scientists fabri - concluded that excited state absorption, cated the fibers by a...topics such as transverse power on the long wavelength side of a switching waves and cross-talk of bista- Fabry -Perot resonance peak at 844 nm, ble

Luminescent properties of Tb3+- doped TeO2-WO3-GeO2 glasses for green laser applications

NASA Astrophysics Data System (ADS)

Subrahmanyam, T.; Rama Gopal, K.; Padma Suvarna, R.; Jamalaiah, B. C.; Vijaya Kumar, M. V.

2018-06-01

Different concentrations of Tb3+ -doped oxyfluoro tellurite (TWGTb) glasses were prepared by conventional melt quenching technique and characterized for green laser applications. The Judd-Ofelt theory was applied to evaluate various spectroscopic and radiative parameters. The TWGTb glasses exhibit 5D3 → 7F5-3 and 5D4 → 7F6-0 transitions when excited at 316 nm radiation. The variation of intensity of 5D4 → 7F5 (Green) and 5D3 → 7F4 (Blue) transitions and the green to blue (IG/IB) intensity ratios were studied as a function of Tb3+ ions concentration. The laser characteristic parameters such as effective bandwidth (Δλeff), stimulated emission cross-section (σe), gain bandwidth (σe × Δλeff) and optical gain (σe × τR) were determined using the three phenomenological Judd-Ofelt intensity parameters. The fluorescence decay profiles of 5D4 metastable level exhibit single-exponential nature for all the samples. Based on the experimental results we suggest that the 1.0 mol% of Tb3+ -doped TWGTb glass could be a suitable laser host material to emit intense green luminescence at 545 nm.

Instantaneous temperature field measurements using planar laser-induced fluorescence.

PubMed

Seitzman, J M; Kychakoff, G; Hanson, R K

1985-09-01

A single-pulse, laser-induced-fluorescence diagnostic for the measurement of two-dimensional temperature fields in combustion flows is described. The method uses sheet illumination from a tunable laser to excite planar laserinduced fluorescence in a stable tracer molecule, seeded at constant mole fraction into the flow field. The temporal resolution of this technique is determined by the laser pulse length. Experimental results are presented for a rodstabilized, premixed methane-air flame, using the Q(1) (22) line of the nitric oxide A(2) Sigma(+) (v = 0) ? X(2)II((1/2))(v = 0) transition (lambda approximately 225.6 nm).

Spectroscopy of Tb3+ ions in monoclinic KLu(WO4)2 crystal application of an intermediate configuration interaction theory

NASA Astrophysics Data System (ADS)

Loiko, Pavel; Volokitina, Anna; Mateos, Xavier; Dunina, Elena; Kornienko, Alexey; Vilejshikova, Elena; Aguiló, Magdalena; Díaz, Francesc

2018-04-01

The spectroscopic properties of Tb3+ ions in monoclinic KLu(WO4)2 double tungstate crystal are studied with polarized light. The absorption spectra in the visible, near- and mid-IR including the transitions to all lower-lying 7FJ (J = 0 … 5) excited states are measured. The maximum absorption cross-section for the 7F6 → 5D4 transition is 3.42 × 10-21 cm2 at 486.7 nm for light polarization E || Nm. The transition probabilities for Tb3+ ions are calculated within the Judd-Ofelt theory modified for the case of an intermediate configuration interaction (ICI). The radiative lifetime of the 5D4 state is 450 μs and the luminescence quantum yield is >90%. The polarized stimulated-emission cross-section spectra for all 5D4 → 7FJ (J = 0 … 6) emission channels are evaluated. The maximum σSE is 11.4 × 10-21 cm2 at 549.4 nm (for E || Nm). Tb3+:KLu(WO4)2 features high transition cross-sections for polarized light being promising for color-tunable visible lasers and imaging.

Stabilizing Microwave Frequency of a Photonic Oscillator

NASA Technical Reports Server (NTRS)

Maleki, Lute; Yu, Nan; Tu, Meirong

2006-01-01

A scheme for stabilizing the frequency of a microwave signal is proposed that exploits the operational characteristics of a coupled optoelectronic oscillator (COEO) and related optoelectronic equipment. An essential element in the scheme is a fiber mode-locked laser (MLL), the optical frequency of which is locked to an atomic transition. In this scheme, the optical frequency stability of the mode-locked laser is transferred to that of the microwave in the same device. Relative to prior schemes for using wideband optical frequency comb to stabilize microwave signals, this scheme is simpler and lends itself more readily to implementation in relatively compact, rugged equipment. The anticipated development of small, low-power, lightweight, highly stable microwave oscillators based on this scheme would afford great benefits in communication, navigation, metrology, and fundamental sciences. COEOs of various designs, at various stages of development, in some cases called by different names, have been described in a number of prior NASA Tech Briefs articles. A COEO is an optoelectronic apparatus that generates both short (picosecond) optical pulses and a steady microwave signal having an ultrahigh degree of spectral purity. The term "coupled optoelectronic" in the full name of such an apparatus signifies that its optical and electronic oscillations are coupled to each other in a single device. The present frequency-stabilization scheme is best described indirectly by describing the laboratory apparatus used to demonstrate it. The apparatus (see figure) includes a COEO that generates a comb-like optical spectrum, the various frequency components of which interfere, producing short optical pulses. This spectrum is centered at a nominal wavelength of 1,560 nm. The spectrum separation of this comb is about 10 GHz, as determined primarily by the length of an optical loop and the bandpass filter in the microwave feedback loop. The optical loop serves as microwave resonator having a very high value of the resonance quality factor (Q). The optical frequency of MLL is then stabilized by locking it to an atomic transition as described below. The COEO contains a tunable 1-nm band-pass optical filter and a piezoelectric-transducer (PZT) drum over which a stretch of fiber is wound. The 1-nm-wide pass band of the filter provides coarse tuning to overlap the frequency comb with the atomic transition frequency. Controlled stretching of the fiber by means of the PZT drum can be used in conjunction with temperature control for locking the laser frequency. To reference to an atomic resonance at 780 nm in this demonstration setup, the optical output of the COEO at 1,560 nm is fed through an erbium-doped-fiber amplifier (EDFA) to a frequency doubler in the form of a periodically poled lithium niobate (PPLN) crystal. The frequency-doubled output is combined with the output of a separate frequency-stabilized diode laser at a photodetector. As described thus far, the two 780-nm laser subsystems are nominally independent of each other and can, therefore, operate at different frequencies. Hence, at the photodetector, the two laser beams interfere, so that the output of the photodetector includes a beat note (a component at the difference between the two laser frequencies).

Low-temperature high-density magneto-optical trapping of potassium using the open 4S{yields}5P transition at 405 nm

DOE Office of Scientific and Technical Information (OSTI.GOV)

McKay, D. C.; Jervis, D.; Fine, D. J.

2011-12-15

We report the laser cooling and trapping of neutral potassium on an open transition. Fermionic {sup 40}K is captured using a magneto-optical trap (MOT) on the closed 4S{sub 1/2}{yields}4P{sub 3/2} transition at 767 nm and then transferred, with high efficiency, to a MOT on the open 4S{sub 1/2}{yields}5P{sub 3/2} transition at 405 nm. Because the 5P{sub 3/2} state has a smaller linewidth than the 4P{sub 3/2} state, the Doppler limit is reduced from 145 {mu}K to 24 {mu}K, and we observe temperatures as low as 63(6) {mu}K. The density of trapped atoms also increases, due to reduced temperature and reducedmore » expulsive light forces. We measure a two-body loss coefficient of {beta}=1.4(1)x10{sup -10} cm{sup 3}/s near saturation intensity, and estimate an upper bound of 8x10{sup -18} cm{sup 2} for the ionization cross section of the 5P state at 405 nm. The combined temperature and density improvement in the 405 nm MOT is a twenty-fold increase in phase-space density over our 767 nm MOT, showing enhanced precooling for quantum gas experiments. A qualitatively similar enhancement is observed in a 405 nm MOT of bosonic {sup 41}K.« less

Control of femtosecond laser interference ejection with angle and polarisation

NASA Astrophysics Data System (ADS)

Roper, David M.; Ho, Stephen; Haque, Moez; Herman, Peter R.

2017-03-01

The nonlinear interactions of femtosecond lasers are driving multiple new application directions for nanopatterning and structuring of thin transparent dielectric films that serve in range of technological fields. Fresnel reflections generated by film interfaces were recently shown to confine strong nonlinear interactions at the Fabry-Perot fringe maxima to generate thin nanoscale plasma disks of 20 to 40 nm thickness stacked on half wavelength spacing, λ/2nfilm, inside a film (refractive index, nfilm). The following phase-explosion and ablation dynamics have resulted in a novel means for intrafilm processing that includes `quantized' half-wavelength machining steps and formation of blisters with embedded nanocavities. This paper presents an extension in the control of interferometric laser processing around our past study of Si3N4 and SiOx thin films at 515 nm, 800 nm, and 1044 nm laser wavelengths. The role of laser polarization and incident angle is explored on fringe visibility and improving interferometric processing inside the film to dominate over interface and / or surface ablation. SiOx thin films of 1 μm thickness on silicon substrates were irradiated with a 515 nm wavelength, 280 fs duration laser pulses at 0° to 65° incident angles. A significant transition in ablation region from complete film removal to structured quantized ejection is reported for p- and s-polarised light that is promising to improve control and expand the versatility of the technique to a wider range of applications and materials. The research is aimed at creating novel bio-engineered surfaces for cell culture, bacterial studies and regenerative medicine, and nanofluidic structures that underpin lab-in-a-film. Similarly, the formation of intrafilm blisters and nanocavities offers new opportunities in structuring existing thin film devices, such as CMOS microelectronics, LED, lab-on-chips, and MEMS.

Faraday effect on the Rb D{sub 1} line in a cell with a thickness of half the wavelength of light

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sargsyan, A., E-mail: sarmeno@mail.ru, E-mail: sargsyanarmen85@gmail.com; Pashayan-Leroy, Y.; Leroy, C.

2016-09-15

The rotation of the radiation polarization plane in a longitudinal magnetic field (Faraday effect) on the D{sub 1} line in atomic Rb vapor has been studied with the use of a nanocell with the thickness L varying in the range of 100–900 nm. It has been shown that an important parameter is the ratio L/λ, where λ = 795 nm is the wavelength of laser radiation resonant with the D{sub 1} line. The best parameters of the signal of rotation of the radiation polarization plane have been obtained at the thickness L = λ/2 = 397.5 nm. The fabricated nanocellmore » had a large region with such a thickness. The spectral width of the signal reached at the thickness L = 397.5 nm is approximately 30 MHz, which is much smaller than the spectral width (≈ 500 MHz) reached with ordinary cells with a thickness in the range of 1–100 mm. The parameters of the Faraday rotation signal have been studied as functions of the temperature of the nanocell, the laser power, and the magnetic field strength. The signal has been reliably detected at the laser power P{sub L} ≥ 1 μW, magnetic field strength B ≥ 0.5 G, and the temperature of the nanocell T ≥ 100°C. It has been shown that the maximum rotation angle of the polarization plane in the longitudinal magnetic field is reached on the F{sub g} = 3 → F{sub e} = 2 transition of the {sup 85}Rb atom. The spectral profile of the Faraday rotation signal has a specific shape with a sharp peak, which promotes its applications. In particular, Rb atomic transitions in high magnetic fields about 1000 G are split into a large number of components, which are completely spectrally resolved and allow the study of the behavior of an individual transition.« less

QED test and nuclear radius determination of helium atom by laser spectroscopy

NASA Astrophysics Data System (ADS)

Pavone, F. S.

1995-01-01

The 23S1-33P0 4He transition at λ = 389 nm is measured with respect to a previously frequency calibrated 87Rb two-photon transition at 2λ = 778 nm. The 4He absolute frequency is 770 732 839 058 (190) kHz, with an accuracy of 2.4 parts in 1010. A Lamb shift value of + 4057.61 (79) MHz, with 600 kHz uncertainty arising from the theoretical position of the 33P0 energy level, is extracted for the 23S1. This value is more than two orders of magnitude more accurate than the current best theoretical predictions. By means of a novel heterodyne spectrometer using only one laser tuned at the atomic frequency, we have measured for the first time the 3He-4He isotope separation for the 23S1-33P0 transition at 389 nm. Our experimental result of 45 394 425 (140) kHz, for the F = 1/2-1/2 3He component, is compared with the theoretical prediction which has similar accuracy and depends also on the rms nuclear radius of 3He. For this we determine a preliminary value of 1.923 (37) fm which shows a slight discrepancy with previous values obtained by extrapolation to zero momentum transfer from high energy scattering measurements.

Optical properties of p–i–n structures based on amorphous hydrogenated silicon with silicon nanocrystals formed via nanosecond laser annealing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Krivyakin, G. K.; Volodin, V. A., E-mail: volodin@isp.nsc.ru; Kochubei, S. A.

Silicon nanocrystals are formed in the i layers of p–i–n structures based on a-Si:H using pulsed laser annealing. An excimer XeCl laser with a wavelength of 308 nm and a pulse duration of 15 ns is used. The laser fluence is varied from 100 (below the melting threshold) to 250 mJ/cm{sup 2} (above the threshold). The nanocrystal sizes are estimated by analyzing Raman spectra using the phonon confinement model. The average is from 2.5 to 3.5 nm, depending on the laser-annealing parameters. Current–voltage measurements show that the fabricated p–i–n structures possess diode characteristics. An electroluminescence signal in the infrared (IR)more » range is detected for the p–i–n structures with Si nanocrystals; the peak position (0.9–1 eV) varies with the laser-annealing parameters. Radiative transitions are presumably related to the nanocrystal–amorphous-matrix interface states. The proposed approach can be used to produce light-emitting diodes on non-refractory substrates.« less

Characteristics of extreme ultraviolet emission from high-Z plasmas

NASA Astrophysics Data System (ADS)

Ohashi, H.; Higashiguchi, T.; Suzuki, Y.; Kawasaki, M.; Suzuki, C.; Tomita, K.; Nishikino, M.; Fujioka, S.; Endo, A.; Li, B.; Otsuka, T.; Dunne, P.; O'Sullivan, G.

2016-03-01

We demonstrate the extreme ultraviolet (EUV) and soft x-ray sources in the 2 to 7 nm spectral region related to the beyond EUV (BEUV) question at 6.x nm and the water window source based on laser-produced high-Z plasmas. Resonance emission from multiply charged ions merges to produce intense unresolved transition arrays (UTAs), extending below the carbon K edge (4.37 nm). An outline of a microscope design for single-shot live cell imaging is proposed based on high-Z plasma UTA source, coupled to multilayer mirror optics.

Heterodyne optical phase-locking of extended-cavity semiconductor lasers at 9 GHz

NASA Astrophysics Data System (ADS)

Santarelli, G.; Clairon, A.; Lea, S. N.; Tino, G. M.

1994-01-01

In order to stimulate atomic velocity-selective Raman transitions on the 852 nm caesium D 2 line in an atomic fountain clock, two extended-cavity diode lasers have been optically phase-locked at a frequency offset of 9.192 GHz. The measured linewidth (fwhm) of the free-running lasers is 50 kHz. The phase-locked loop bandwidth, evaluated by observing the frequency noise spectrum, is 3.7 MHz and the phase error variance is found to be no more than 4 × 10 -3 rad 2.

Programmable frequency reference for subkilohertz laser stabilization by use of persistent spectral hole burning.

PubMed

Sellin, P B; Strickland, N M; Carlsten, J L; Cone, R L

1999-08-01

We report what is believed to be the first demonstration of laser frequency stabilization directly to persistent spectral holes in a solid-state material. The frequency reference material was deuterated CaF(2): Tm(3+) prepared with 25-MHz-wide persistent spectral holes on the H(6)(3)?H(4)(3) transition at 798 nm. The beat frequency between two lasers that were independently locked to persistent spectral holes in separate crystal samples showed typical root Allan variances of 780+/-120Hz for 20-50-ms integration times.

Room-temperature subnanosecond waveguide lasers in Nd:YVO4 Q-switched by phase-change VO2: A comparison with 2D materials

PubMed Central

Nie, Weijie; Li, Rang; Cheng, Chen; Chen, Yanxue; Lu, Qingming; Romero, Carolina; Vázquez de Aldana, Javier R.; Hao, Xiaotao; Chen, Feng

2017-01-01

We report on room-temperature subnanosecond waveguide laser operation at 1064 nm in a Nd:YVO4 crystal waveguide through Q-switching of phase-change nanomaterial vanadium dioxide (VO2). The unique feature of VO2 nanomaterial from the insulating to metallic phases offers low-saturation-intensity nonlinear absorptions of light for subnanosecond pulse generation. The low-loss waveguide is fabricated by using the femtosecond laser writing with depressed cladding geometry. Under optical pump at 808 nm, efficient pulsed laser has been achieved in the Nd:YVO4 waveguide, reaching minimum pulse duration of 690 ps and maximum output average power of 66.7 mW. To compare the Q-switched laser performances by VO2 saturable absorber with those based on two-dimensional materials, the 1064-nm laser pulses have been realized in the same waveguide platform with either graphene or transition metal dichalcogenide (in this work, WS2) coated mirror. The results on 2D material Q-switched waveguide lasers have shown that the shortest pulses are with 22-ns duration, whilst the maximum output average powers reach ~161.9 mW. This work shows the obvious difference on the lasing properties based on phase-change material and 2D materials, and suggests potential applications of VO2 as low-cost saturable absorber for subnanosecond laser generation. PMID:28383017

Graphite to ultrafine nanocrystalline diamond phase transition model and growth restriction mechanism induced by nanosecond laser processing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ren, X. D., E-mail: renxd@mail.ujs.edu.cn; Liu, R.; Zheng, L. M.

2015-10-05

To have a clear insight into nanocrystal growth from graphite to diamond upon high energy pulsed laser irradiation of graphite suspension, synthesis of ultrafine nanocrystalline diamonds with laser energy set up from 0.3 J to 12 J, repetition rate of 10 Hz has been studied. The method allows synthesizing ultrafine nanocrystalline particles continuously at the ambient temperature and normal pressure. The particle size is shown independent of laser energy, which is ultrafine and ranges in 2–6 nm. The theoretical grown size of nano-diamonds is found in well agreement with the experiment results. Four kinds of production were found: nano-diamond, spherical carbon nano-particles, flocculent amorphousmore » carbon, and graphene nano-ribbon rolls. A solid-vapor-plasma-liquid coexistence model describing phase transition from graphite to diamond induced by nanosecond laser processing was proposed. Graphene nano-ribbon rolls might be the intermediate phase in the conversion from graphite to diamond.« less

Electro-Optical Properties of Polymer Blends: Lasing, Electroluminescence and Photophysics

DTIC Science & Technology

2007-02-01

34- Phenylenevinylene" (Cirpan/Rathnayake/Lahti/Karasz) 16. Chem. Mater.: "Single-Molecule and Bulk Luminescence Studies of the Green Emission Band in 2,7- Bis...providing emission from the triplet state with a 100% theoretical yield. These electronic transitions of lanthanides result from different electronic...referred to above. Luminescence spectra and luminescence decays were recorded with a Thermo Laser Science pulsed nitrogen laser ( Aem =3 3 7 .1 nm; < 4 ns

LPTF frequency synthesis chain: Results and improvement for the near future

DOE Office of Scientific and Technical Information (OSTI.GOV)

Touahri, D.; Zondy, J.J.; Acef, O.

1994-12-31

We have measured the frequency of the He-Ne/12 laser starting from the Cs referenced CO{sub 2}/OsO{sub 4} laboratory standard. As the laser diode stabilized on the two-photon transition in Rb seems to be a suitable reference for spectroscopic studies. (H, He ... ) and a promising standard, we are modifying our chain in order to measure frequencies around 780 nm and specially the Rb one.

Observation of strong amplification at 8.8 nm in the TCE scheme by a table-top pumping system

NASA Astrophysics Data System (ADS)

Kawachi, Tetsuya; Tanaka, Momoko; Sasaki, Akira; Kishimoto, Maki; Nishiuchi, Mamiko; Yasuike, Kazuhito; Hasegawa, Noboru; Kilpio, Alexander V.; Lu, Peixiang; Tai, Renzhong

2002-11-01

We observed strong amplification of the transition of 4d 4p, J = 0 1 (the transition from (3d3/2, 4d3/2)0 to (3d3/2, 4p1/2)1) of the Ni-like lanthanum (La) ions at a wavelength of 8.8 nm pumped by a compact CPA Nd:Glass laser light at a wavelength of 1.053 mum with a pumping energy of 18 J. The experimental gain coefficient and the achieved gain-length product was 14.5 cm-1 and 7.7, respectively. In this experiment, the pumping laser pulse consisted of a pre-pulse with a duration of 200 ps and a 7ps-duration main pulse, separated by 250 ps. A hydrodynamics simulation coupled with a collisional-radiative model showed that the present experimental condition generated a pre-formed plasma with small volume and made it possible by the main pulse to heat the high density region effectively.

Optical properties of Sm3+ -doped TeO2sbnd WO3sbnd GeO2 glasses for solid state lasers

NASA Astrophysics Data System (ADS)

Subrahmanyam, T.; Gopal, K. Rama; Suvarna, R. Padma; Jamalaiah, B. Chinna; Rao, Ch Srinivasa

2018-03-01

Sm3+ -doped oxyfluoride tellurite-tungsten (TWGSm) glasses were prepared by conventional melt quenching method. The optical properties were investigated through photoluminescence excitation, emission and luminescence decay analysis. The optical band gap energy was determined as ∼3.425 eV for 1.0 mol% of Sm3+ -doped TWGSm glass. Upon 404 nm excitation, the TWGSm glasses emit luminescence through 4G5/2 → 6H5/2 (563 nm), 4G5/2 → 6H7/2 (600 nm), 4G5/2 → 6H9/2 (645 nm) and 4G5/2 → 6H11/2 (705 nm) transitions. The Judd-Ofelt analysis was performed using absorption spectrum and obtained radiative parameters were used to estimate the laser characteristics of present glasses. The concentration of Sm3+ has been optimized as 1.0 mol% for efficient luminescence. The luminescence decay of 4G5/2 emission level was studied by monitoring the emission and excitation wavelengths at 600 and 404 nm, respectively. The experimental lifetime of 4G5/2 level was decrease with increase of Sm3+ concentration. The 1.0 mol% of Sm3+ -doped TWGSm glass could be the best choice for solid state visible lasers to emit orange luminescence.

Tuning excitation laser wavelength for secondary resonance in low-intensity phase-selective laser-induced breakdown spectroscopy for in-situ analytical measurement of nanoaerosols

NASA Astrophysics Data System (ADS)

Xiong, Gang; Li, Shuiqing; Tse, Stephen D.

2018-02-01

In recent years, a novel low-intensity phase-selective laser-induced breakdown spectroscopy (PS-LIBS) technique has been developed for unique elemental-composition identification of aerosolized nanoparticles, where only the solid-phase nanoparticles break down, forming nanoplasmas, without any surrounding gas-phase breakdown. Additional work has demonstrated that PS-LIBS emissions can be greatly enhanced with secondary resonant excitation by matching the excitation laser wavelength with an atomic transition line in the formed nanoplasma, thereby achieving low limits of detection. In this work, a tunable dye laser is employed to investigate the effects of excitation wavelength and irradiance on in-situ PS-LIBS measurements of TiO2 nanoaerosols. The enhancement factor by resonant excitation can be 220 times greater than that for non-resonant cases under similar conditions. Moreover, the emitted spectra are unique for the selected resonant transition lines for a given element, suggesting the potential to make precise phase-selective and analyte-selective measurements of nanoparticles in a multicomponent multiphase system. The enhancement factor by resonant excitation is highly sensitive to excitation laser wavelength, with narrow excitation spectral windows, i.e., 0.012 to 0.023 nm (FWHM, full width at half maximum) for Ti (I) neutral atomic lines, and 0.051 to 0.139 nm (FWHM) for Ti (II) single-ionized atomic lines. Boltzmann analysis of the emission intensities, temporal response of emissions, and emission dependence on excitation irradiance are investigated to understand aspects of the generated nanoplasmas such as temperature, local thermodynamic equilibrium (LTE), and excitation mechanism.

Observation of the 162Dy-164Dy Isotope Shift for the 0 → 16 717.79 cm-1 Optical Transition.

PubMed

Nardin Barreta, Luiz Felipe; Victor, Alessandro Rogério; Bueno, Patrícia; Dos Santos, Jhonatha Ricardo; da Silveira, Carlos Alberto Barbosa; Neri, José Wilson; Neto, Jonas Jakutis; Sbampato, Maria Esther; Destro, Marcelo Geraldo

2017-08-01

In this work, we report a newly observed isotope shift between 162 Dy and 164 Dy isotopes for the 0 → 16 717.79 cm -1 (598.003 nm) optical transition. We compared the newly observed results against two other lines (597.452 nm and 598.859 nm), which we measured in this work, and were already reported in the literature. The newly observed 162-164 Dy isotope shift, shows at least a 20% larger isotope shift than the isotope shifts for the other two lines investigated. The larger 162-164 isotope shift observed for the 598.003 nm line could lead to an increased isotope selectivity for atomic vapor laser isotope separation (AVLIS). Hence, this line could be a good choice for application in AVLIS. Experimental data available in the literature for the 597.452 nm and 598.859 nm lines, enabled us to perform simulations of spectra for both lines, in order to confirm the accuracy of our experimental measurements.

Near-Resonant Raman Amplification in the Rotational Quantum Wave Packets of Nitrogen Molecular Ions Generated by Strong Field Ionization

NASA Astrophysics Data System (ADS)

Liu, Zhaoxiang; Yao, Jinping; Chen, Jinming; Xu, Bo; Chu, Wei; Cheng, Ya

2018-02-01

The generation of laserlike narrow bandwidth emissions from nitrogen molecular ions (N2+ ) generated in intense near- and mid infrared femtosecond laser fields has aroused much interest because of the mysterious physics underlying such a phenomenon. Here, we perform a pump-probe measurement on the nonlinear interaction of rotational quantum wave packets of N2+ generated in midinfrared (e.g., at a wavelength centered at 1580 nm) femtosecond laser fields with an ultrashort probe pulse whose broad spectrum overlaps both P - and R -branch rotational transition lines between the electronic states N2+(B2Σu+,v'=0 ) and N2+(X2Σg+,v =0 ) . The results indicate the occurrence of highly efficient near-resonant stimulated Raman scattering in the quantum wave packets of N2+ ions generated in strong laser fields in the midinfrared region, of which the underlying mechanism is different from that of the air lasers generated in atmospheric environment when pumping with 800 nm intense pulses.

Random lasing in Nd{sup 3+} doped potassium gadolinium tungstate crystal powder

DOE Office of Scientific and Technical Information (OSTI.GOV)

Moura, André L., E-mail: andre.moura@fis.ufal.br; Departamento de Física, Universidade Federal de Pernambuco, 50670-901 Recife, PE; Fewo, Serge I.

2015-02-28

Random laser (RL) emission in Nd{sup 3+} doped potassium gadolinium tungstate—KGd(WO{sub 4}){sub 2}:Nd{sup 3+}—crystal powder is demonstrated. The powder was excited at 813 nm in resonance with the Nd{sup 3+} transition {sup 4}I{sub 9/2}→{sup 4}F{sub 5/2}. RL emission at 1067 nm due to the {sup 4}F{sub 3/2}→{sup 4}I{sub 11/2} transition was observed and characterized. An intensity threshold dependent on the laser spot area and bandwidth narrowing from ≈2.20 nm to ≈0.40 nm were observed and measured. For a beam spot area of 0.4 mm{sup 2}, a RL threshold of 6.5 mJ/mm{sup 2} (90 MW/cm{sup 2}) was determined. For excitation intensity smaller than the RL threshold, only spontaneousmore » emission from level {sup 4}F{sub 3/2} with decay time in the tens microsecond range was observed, but for excitation above the RL threshold, significant shortening of excited level lifetime, characteristic of a stimulated process was found. The overall characteristics measured show that KGd(WO{sub 4}){sub 2}:Nd{sup 3+} is an efficient material for operation of solid state RLs in the near-infrared.« less

Spectroscopy of TaN in Support of Fundamental Physics

NASA Astrophysics Data System (ADS)

Mawhorter, Richard; Sharfi, David; Kim, Yongrak; Kokkin, Damian; Bouchard, Jacob; Steimle, Timothy

2016-05-01

Tantalum nitride, TaN, has been recently identified as a leading candidate for extending the study of T, P-odd effects in the nuclear realm to include proton, neutron, and quark electric dipole moments (EDM) and beyond. This is primarily due to enhancements in the interaction of electrons with the nuclear magnetic quadrupole moment (MQM) and the resulting parity-violating effects. Study of the dispersed laser induced fluorescence resulting from the excitation of the 17570.80 (Ω = 0+) , 18427.38 (Ω = 0+) , 19216.80 (Ω = 1), and 19396.78 (Ω = 1) bands above the X1Σ+ (v = 0) ground state of TaN near 569 nm, 543 nm, 520 nm, and 515 nm has enabled a determination of the branching ratios and transition dipole moments of all 4 states. Radiative lifetimes of 454(32) ns, 479(12) ns, 333(4) ns, and 480(17) ns respectively were measured from an analysis of the fluorescence decay curves, and potential optical pumping approaches for both populating and detecting the parity-violation sensitive 3Δ1 state are proposed. Further experiments using CW laser excitation have enabled the observation of the hyperfine structure of several bands in the gateway 18427.38 (Ω = 0+) to X1Σ+ (v = 0) transition, and analysis of these complex spectra is underway. DK, JB, and TS acknowledge support from NSF CHE-1265885, as do RM, DS, and YK from Pomona College.

Infrared nanosecond laser-metal ablation in atmosphere: Initial plasma during laser pulse and further expansion

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wu, Jian; Wei, Wenfu; Li, Xingwen

2013-04-22

We have investigated the dynamics of the nanosecond laser ablated plasma within and after the laser pulse irradiation using fast photography. A 1064 nm, 15 ns laser beam was focused onto a target made from various materials with an energy density in the order of J/mm{sup 2} in atmosphere. The plasma dynamics during the nanosecond laser pulse were observed, which could be divided into three stages: fast expansion, division into the primary plasma and the front plasma, and stagnation. After the laser terminated, a critical moment when the primary plasma expansion transited from the shock model to the drag modelmore » was resolved, and this phenomenon could be understood in terms of interactions between the primary and the front plasmas.« less

Thermal evaluation of laser exposures in an in vitro retinal model by microthermal sensing

NASA Astrophysics Data System (ADS)

Choi, Tae Y.; Denton, Michael L.; Noojin, Gary D.; Estlack, Larry E.; Shrestha, Ramesh; Rockwell, Benjamin A.; Thomas, Robert; Kim, Dongsik

2014-09-01

A temperature detection system using a micropipette thermocouple sensor was developed for use within mammalian cells during laser exposure with an 8.6-μm beam at 532 nm. We have demonstrated the capability of measuring temperatures at a single-cell level in the microscale range by inserting micropipette-based thermal sensors of size ranging from 2 to 4 μm into the membrane of a live retinal pigment epithelium (RPE) cell subjected to a laser beam. We setup the treatment groups of 532-nm laser-irradiated single RPE cell and in situ temperature recordings were made over time. Thermal profiles are given for representative cells experiencing damage resulting from exposures of 0.2 to 2 s. The measured maximum temperature rise for each cell ranges from 39 to 73°C the RPE cells showed a signature of death for all the cases reported herein. In order to check the cell viability, real-time fluorescence microscopy was used to identify the transition of pigmented RPE cells between viable and damaged states due to laser exposure.

Laser ablated copper plasmas in liquid and gas ambient

NASA Astrophysics Data System (ADS)

Kumar, Bhupesh; Thareja, Raj K.

2013-05-01

The dynamics of copper ablated plasma plumes generated using laser ablation of copper targets in both liquid (de-ionized water) and gas (air) ambients is reported. Using time and space resolved visible emission spectroscopy (450-650 nm), the plasma plumes parameters are investigated. The electron density (ne) determined using Stark broadening of the Cu I (3d104d1 2D3/2-3d104p1 2P3/2 at 521.8 nm) line is estimated and compared for both plasma plumes. The electron temperature (Te) was estimated using the relative line emission intensities of the neutral copper transitions. Field emission scanning electron microscopy and energy dispersive x-ray spectral analysis of the ablated copper surface indicated abundance of spherical nanoparticles in liquid while those in air are amalgamates of irregular shapes. The nanoparticles suspended in the confining liquid form aggregates and exhibit a surface plasmon resonance at ˜590 nm.

Generation of multiple spectral bands in a diode-pumped self-mode-locked Nd:YAP laser

NASA Astrophysics Data System (ADS)

Huang, Y. J.; Tzeng, Y. S.; Cho, H. H.; Chen, Y. F.; Chen, W. D.; Zhang, G.; Chen, T. C.

2016-02-01

A single- and multispectral-band diode end-pumped self-mode-locked Nd:YAP laser is originally demonstrated with an intracavity etalon to properly control the gain-to-loss ratios among the intermanifold lines on the 4F3/2  →  4I11/2 transition level. With a pulse repetition rate of 5.07 GHz, the shortest pulse durations under the single-spectral-band operation are achieved to be 11.1 ps at 1073 nm, 10.9 ps at 1080 nm, and 15.1 ps at 1084 nm, respectively. Moreover, the temporal overlapping of the multispectral-band pulses is experimentally found to lead to the generation of an intensity fringe pattern in the autocorrelation trace with the optical-beat frequency reaching several terahertz. A simple mathematical model is developed to elucidate the formation of a train of optical-beat pulses.

Heat-sink free CW operation of injection microdisk lasers grown on Si substrate with emission wavelength beyond 1.3  μm.

PubMed

Kryzhanovskaya, Natalia; Moiseev, Eduard; Polubavkina, Yulia; Maximov, Mikhail; Kulagina, Marina; Troshkov, Sergey; Zadiranov, Yury; Guseva, Yulia; Lipovskii, Andrey; Tang, Mingchu; Liao, Mengya; Wu, Jiang; Chen, Siming; Liu, Huiyun; Zhukov, Alexey

2017-09-01

High-performance injection microdisk (MD) lasers grown on Si substrate are demonstrated for the first time, to the best of our knowledge. Continuous-wave (CW) lasing in microlasers with diameters from 14 to 30 μm is achieved at room temperature. The minimal threshold current density of 600  A/cm 2 (room temperature, CW regime, heatsink-free uncooled operation) is comparable to that of high-quality MD lasers on GaAs substrates. Microlasers on silicon emit in the wavelength range of 1320-1350 nm via the ground state transition of InAs/InGaAs/GaAs quantum dots. The high stability of the lasing wavelength (dλ/dI=0.1  nm/mA) and the low specific thermal resistance of 4×10 -3 °C×cm 2 /W are demonstrated.

Thermally and optically tunable lasing properties from dye-doped holographic polymer dispersed liquid crystal in capillaries

NASA Astrophysics Data System (ADS)

Chen, Maozhou; Dai, Haitao; Wang, Dongshuo; Yang, Yue; Luo, Dan; Zhang, Xiaodong; Liu, Changlong

2018-03-01

In this paper, we investigated tunable lasing properties from the dye-doped holographic polymer dispersed liquid crystal (HPDLC) gratings in capillaries with thermal and optical manners. The thermally tunable range of the lasing from the dye-doped HPDLC reached 8.60 nm with the temperature ranging from 23 °C to 50 °C. The optically tunable laser emission was achieved by doping azo-dye in HPDLC. The transition of azo-dye from trans- to cis-state could induce the reorientation of LC molecules after UV light irradiation, which resulted in the variation of refractive index contrast of LC-rich/polymer-rich layer in HPDLC. Experimentally, the emission wavelength of lasing showed a blueshift (about 2 nm) coupled with decreasing output intensities. The tunable laser based on HPDLC may enable more applications in laser displays, optical communication, biosensors, etc.

Progress to a Gallium-Arsenide Deep-Center Laser

PubMed Central

Pan, Janet L.

2009-01-01

Although photoluminescence from gallium-arsenide (GaAs) deep-centers was first observed in the 1960s, semiconductor lasers have always utilized conduction-to-valence-band transitions. Here we review recent materials studies leading to the first GaAs deep-center laser. First, we summarize well-known properties: nature of deep-center complexes, Franck-Condon effect, photoluminescence. Second, we describe our recent work: insensitivity of photoluminescence with heating, striking differences between electroluminescence and photoluminescence, correlation between transitions to deep-states and absence of bandgap-emission. Room-temperature stimulated-emission from GaAs deep-centers was observed at low electrical injection, and could be tuned from the bandgap to half-the-bandgap (900–1,600 nm) by changing the electrical injection. The first GaAs deep-center laser was demonstrated with electrical injection, and exhibited a threshold of less than 27 mA/cm2 in continuous-wave mode at room temperature at the important 1.54 μm fiber-optic wavelength. This small injection for laser action was explained by fast depopulation of the lower state of the optical transition (fast capture of free holes onto deep-centers), which maintains the population inversion. The evidence for laser action included: superlinear L-I curve, quasi-Fermi level separations satisfying Bernard-Duraffourg’s criterion, optical gains larger than known significant losses, clamping of the optical-emission from lossy modes unable to reach laser action, pinning of the population distribution during laser action.

Possibility of Recombination Gain Increase in CV Ions at 4.0 nm Via Coherence

NASA Astrophysics Data System (ADS)

Luo, Y.; Morozov, A.; Gordon, D.; Sprangle, P.; Svidzinsky, A.; Xia, H.; Scully, M.; Suckewer, S.

This paper is about the recent experimental results on amplification of the CV line in the "water window" at 4.03 nm from resonance transition to the ground level of He-like ions in recombination scheme. The indication of the amplification of the CV line has been observed when an elongated narrow plasma channel was created, where high intensity 100 fs beams, optimal for creating CV ions in high density plasma, was propagated up to 0.5-0.6 mm. Without channeling the effective plasma length was much shorter and there was no indication of amplification.The large interest in gain generation in He-like ions in the transition to ground state is due to the possibility of applying a recently developed theory of Lasing Without Inversion (LWI) in XUV and X-ray regions to largely increase the gain for such transitions. The presented results of the indication of CV line amplifications are being discussed from the point of view of using LWI as a superradiance gain increase, hence to construct a very compact soft X-ray laser in the "water window".The last part of the paper is related to the application of the ultra-intensive fs plasma laser, which is currently in the process of development by using stimulated Raman backscattering (SRBS) to create a plasma amplifier and compressor, as the pump for compact laser operating in the "water window" and also at shorter wavelengths.

Selective reflection of laser radiation from submicron layers of Rb and Cs atomic vapors: Applications in atomic spectroscopy

NASA Astrophysics Data System (ADS)

Klinger, E.; Sargsyan, A.; Leroy, C.; Sarkisyan, D.

2017-10-01

We studied selective reflection (SR) of laser radiation from a window of a nanocell with thickness L λ 1,2/2 filled with Rb and Cs atoms, where λ 1 = 780 nm and λ 2 = 852 nm are the wavelengths resonant with the D 2 laser lines for Rb and Cs, respectively. It is demonstrated that the negative derivative of the SR signal profile for L > λ/2 changes to the positive one for L < λ/2. It is shown that the real-time formation of the SR signal profile derivative (SRD) with the spectral width 30-40 MHz and located at the atomic transition is, in particular, a convenient frequency marker of D 2 transitions in Rb and Cs. The amplitudes of SRD signals are proportional to the atomic transition probabilities. A comparison with the known saturated absorption (SA) method demonstrated a number of advantages, such as the absence of cross-over resonances in the SRD spectrum, the simplicity of realization, a low required power, etc. An SRD frequency marker also operates in the presence of the Ne buffer gas at a pressure of 6 Torr, which allowed us to determine the Ne-Rb collisional broadening, whereas the SA method is already inapplicable at buffer gas pressures above 0.1 Torr. The realization simplicity makes the SRD method a convenient tool for atomic spectroscopy. Our theoretical model well describes the SRD signal.

Design concepts of monolithic metamorphic vertical-cavity surface-emitting lasers for the 1300–1550 nm spectral range

DOE Office of Scientific and Technical Information (OSTI.GOV)

Egorov, A. Yu., E-mail: anton@beam.ioffe.ru; Karachinsky, L. Ya.; Novikov, I. I.

Possible design concepts for long-wavelength vertical-cavity surface-emitting lasers for the 1300–1550 nm spectral range on GaAs substrates are suggested. It is shown that a metamorphic GaAs–InGaAs heterostructure with a thin buffer layer providing rapid transition from the lattice constant of GaAs to that of In{sub x}Ga{sub 1–x}As with an indium fraction of x < 0.3 can be formed by molecular-beam epitaxy. Analysis by transmission electron microscopy demonstrated the effective localization of mismatch dislocations in the thin buffer layer and full suppression of their penetration into the overlying InGaAs metamorphic layer.

Near Infrared Luminescence Properties of Mn(5+): Ca5(PO4)3F

NASA Technical Reports Server (NTRS)

Davis, Valetta R.; Hoemmerich, Uwe; Loutts, George B.

1997-01-01

We report a spectroscopic investigation of Mn(5+) doped Ca5(PO4)(sub 3)F or FAP. Mn(5+) doped crystals have recently attracted world wide attention for potential solid-state laser applications. Following optical excitation of Mn: FAP with the 600 nm output of a Nd: YAG OPO laser system, we observed a strong near infrared luminescence centered at around 1150 nm. The room temperature luminescence decay time was measured to be approximately 635 microseconds. We attribute the infrared luminescence to the(1)E yields (3)A2 transition of tetrahedrally coordinated Mn5+ ions located in a strong crystal field environment. Absorption, luminescence and lifetime data of Mn: FAP will be presented and discussed.

Laser heating dynamics and glow spectra of carbon-, titanium- and erbium-containing optothermal fibre converters for laser medicine

NASA Astrophysics Data System (ADS)

Belikov, A. V.; Skrypnik, A. V.

2017-07-01

Titanium- and erbium-containing optothermal fibre converters of laser radiation mounted at the distal end of quartz-quartz optical fibre are discussed for the first time. Technology of fabricating such converters is described. Carbon-containing converters are also considered. The laser heating dynamics of the converters and the glow spectra are studied by irradiating converters of each type by a 980 ± 10 nm semiconductor laser with an average power up to 4 W. It is shown that alongside with broadband thermal radiation accompanying the laser heating of all three types of converters in the temperature range 600-1100 °C, only in the spectrum of the erbium-containing converter the intense bands with the maxima at wavelengths 493, 523, 544, 660, and 798 nm, corresponding to the erbium radiative transitions 4F7/2 → 4I15/2, 2H11/2 → 4I15/2, 4S3/2 → 4I15/2, 4F9/2 → 4I15/2 and 4I9/2 → 4I15/2, respectively, are present. Such converters can be used in laser medicine for tissue surgery as well as in procedures combining laser, thermal, biostimulation or photodynamic action.

Instantaneous imaging of ozone in a gliding arc discharge using photofragmentation laser-induced fluorescence

NASA Astrophysics Data System (ADS)

Larsson, Kajsa; Hot, Dina; Gao, Jinlong; Kong, Chengdong; Li, Zhongshan; Aldén, Marcus; Bood, Joakim; Ehn, Andreas

2018-04-01

Ozone vapor, O3, is here visualized in a gliding arc discharge using photofragmentation laser-induced fluorescence. Ozone is imaged by first photodissociating the O3 molecule into an O radical and a vibrationally hot O2 fragment by a pump photon. Thereafter, the vibrationally excited O2 molecule absorbs a second (probe) photon that further transits the O2-molecule to an excited electronic state, and hence, fluorescence from the deexcitation process in the molecule can be detected. Both the photodissociation and excitation processes are achieved within one 248 nm KrF excimer laser pulse that is formed into a laser sheet and the fluorescence is imaged using an intensified CCD camera. The laser-induced signal in the vicinity of the plasma column formed by the gliding arc is confirmed to stem from O3 rather than plasma produced vibrationally hot O2. While both these products can be produced in plasmas a second laser pulse at 266 nm was utilized to separate the pump- from the probe-processes. Such arrangement allowed lifetime studies of vibrationally hot O2, which under these conditions were several orders of magnitude shorter than the lifetime of plasma-produced ozone.

Up-conversion luminescence of Er3+ ions in lead-free germanate glasses under 800 nm and 980 nm cw diode laser excitation

NASA Astrophysics Data System (ADS)

Janek, J.; Lisiecki, R.; Ryba-Romanowski, W.; Pisarska, J.; Pisarski, W. A.

2017-12-01

Up-conversion luminescence spectra of Er3+ ions in multicomponent oxyfluoride glasses GeO2 - BaO - BaF2 - Ga2O3 - Er2O3 were examined. It was found that the up-conversion luminescence spectra of Er3+ are dependent on pumping wavelengths. The spectra recorded upon the excitation at 800 nm contained an intense green up-conversion luminescence corresponding to the 2H11/2,4S3/2 → 4I15/2 transitions and a very weak red luminescence related to the 4F9/2 - 4I15/2 transition. In spectra recorded upon 980 nm excitation the contribution of the red luminescence was markedly higher. The interaction mechanisms involved in up-conversion processes are proposed and observed dependence of intensity of up-converted luminescence on excitation power is discussed. The experimental results suggest that Er3+ singly doped lead-free oxyfluoride germanate glass is useful for up-conversion luminescence applications.

Study of laser cooling in deep optical lattice: two-level quantum model

NASA Astrophysics Data System (ADS)

Prudnikov, O. N.; Il'enkov, R. Ya.; Taichenachev, A. V.; Yudin, V. I.; Rasel, E. M.

2018-01-01

We study a possibility of laser cooling of 24Mg atoms in deep optical lattice formed by intense off-resonant laser field in a presence of cooling field resonant to narrow (3s3s) 1 S 0 → (3s3p)3 P 1 (λ = 457 nm) optical transition. For description of laser cooling with taking into account quantum recoil effects we consider two quantum models. The first one is based on direct numerical solution of quantum kinetic equation for atom density matrix and the second one is simplified model based on decomposition of atom density matrix over vibration states in the lattice wells. We search cooling field intensity and detuning for minimum cooling energy and fast laser cooling.

Experimental and theoretical study on emission spectra of a nitrogen photoionized plasma induced by intense EUV pulses

NASA Astrophysics Data System (ADS)

Saber, Ismail; Bartnik, Andrzej; Skrzeczanowski, Wojciech; Wachulak, Przemyslaw; Jarocki, Roman; Fiedorowicz, Henryk; Limpouch, Jiri

2018-01-01

Spectral lines of low-temperature nitrogen photoionized plasma were investigated. The photoionized plasma was created in the result of irradiation N2 gas using laser plasma EUV radiation pulses. The source was based on a 10J/10ns Nd:YAG (λ = 1064 nm) laser system and a gas puff target. The EUV radiation pulses were collected and focused using a grazing incidence multifoil EUV collector. The emission spectra were measured in the ultraviolet and visible (UV/Vis) range. It was found that the plasma emission lines in the lower region of the UV range are relativley weak. Nonetheless, a part of the spectra contains strong molecular band in the 300 - 430 nm originated from second positive and first negative systems band transitions of nitrogen. These molecular band transitions were identified using a code for study the diatomic molecules, LIFBASE. The vibrational band of Δv = 0 and ±1 transitions were significantly populated than of that with Δv = ±2 and 3 transitions. A comparison of the calculated and measured spectrum is presented. With an assumption of a local thermodynamic equilibrium (LTE), the vibrational temperature was determined from the integrated band intensities with the help of the Boltzmann plot method and compared to the temperature predicted by SPECAIR and LIFBASE simulations. A summary of the results and the variations in the vibrational temperatures was discussed.

DURIP: Fast Oscilloscope and Detectors for Air Laser Research

DTIC Science & Technology

2015-01-01

TEKTRONIX DPO73304D, 33 GHz Digital Phosphor Oscilloscope; 4 analog channels DPO70604C, 6 GHz Digital Phosphor Oscilloscope; 4 analog channels...when we focus in air intense UV pulses resonantly with two-photon transitions in atomic oxygen or nitrogen. The UV pump pulse (or an...two-­‐photon   UV  pumping  at  226nm  for  oxygen,  and  at  207  or  211nm  for   nitrogen   is   followed   by

Polarization spectroscopy of atomic erbium in a hollow cathode lamp

NASA Astrophysics Data System (ADS)

Ang'ong'a, Jackson; Gadway, Bryce

2018-02-01

In this work we perform polarization spectroscopy of erbium atoms in a hollow cathode lamp (HCL). We review the theory behind Doppler-free polarization spectroscopy, theoretically model the expected erbium polarization spectra, and compare the numerically calculated spectra to our experimental data. We further analyze the dependence of the measured spectra on the HCL current and the peak intensities of our pump and probe lasers to determine conditions. Applications include wavelength stabilization of diode laser radiation to the 400.91 nm erbium transition.

Analysis of geological materials containing uranium using laser-induced breakdown spectroscopy (LIBS)

NASA Astrophysics Data System (ADS)

Barefield, James E.; Judge, Elizabeth J.; Campbell, Keri R.; Colgan, James P.; Kilcrease, David P.; Johns, Heather M.; Wiens, Roger C.; McInroy, Rhonda E.; Martinez, Ronald K.; Clegg, Samuel M.

2016-06-01

Laser induced breakdown spectroscopy (LIBS) is a rapid atomic emission spectroscopy technique that can be configured for a variety of applications including space, forensics, and industry. LIBS can also be configured for stand-off distances or in-situ, under vacuum, high pressure, atmospheric or different gas environments, and with different resolving-power spectrometers. The detection of uranium in a complex geological matrix under different measurement schemes is explored in this paper. Although many investigations have been completed in an attempt to detect and quantify uranium in different matrices at in-situ and standoff distances, this work detects and quantifies uranium in a complex matrix under Martian and ambient air conditions. Investigation of uranium detection using a low resolving-power LIBS system at stand-off distances (1.6 m) is also reported. The results are compared to an in-situ LIBS system with medium resolving power and under ambient air conditions. Uranium has many thousands of emission lines in the 200-800 nm spectral region. In the presence of other matrix elements and at lower concentrations, the limit of detection of uranium is significantly reduced. The two measurement methods (low and high resolving-power spectrometers) are compared for limit of detection (LOD). Of the twenty-one potential diagnostic uranium emission lines, seven (409, 424, 434, 435, 436, 591, and 682 nm) have been used to determine the LOD for pitchblende in a dunite matrix using the ChemCam test bed LIBS system. The LOD values determined for uranium transitions in air are 409.013 nm (24,700 ppm), 424.167 nm (23,780 ppm), 434.169 nm (24,390 ppm), 435.574 nm (35,880 ppm), 436.205 nm (19,340 ppm), 591.539 nm (47,310 ppm), and 682.692 nm (18,580 ppm). The corresponding LOD values determined for uranium transitions in 7 Torr CO2 are 424.167 nm (25,760 ppm), 434.169 nm (40,800 ppm), 436.205 nm (32,050 ppm), 591.539 nm (15,340 ppm), and 682.692 nm (29,080 ppm). The LOD values determine for uranium emission lines using the medium resolving power (10,000 λ/Δλ) LIBS system for the dunite matrix in air are 409.013 nm (6120 ppm), 424.167 nm (5356 ppm), 434.169 nm (5693 ppm), 435.574 nm (6329 ppm), 436.205 nm (2142 ppm), and 682.692 nm (10,741 ppm). The corresponding LOD values determined for uranium transitions in a SiO2 matrix are 409.013 nm (272 ppm), 424.167 nm (268 ppm), 434.169 nm (402 ppm), 435.574 nm (1067 ppm), 436.205 nm (482 ppm), and 682.692 nm (720 ppm). The impact of spectral resolution, atmospheric conditions, matrix elements, and measurement distances on LOD is discussed. The measurements will assist one in selecting the proper system components based upon the application and the required analytical performance.

Development of very compact soft X-ray lasers

NASA Astrophysics Data System (ADS)

Korobkin, Dmitriy Vladlenovich

1999-10-01

A powerful subpicosecond laser system, based on solid state (Ti:Al 2O3) front end and gas excimer (KrF*) amplifiers, has been developed. It is capable of producing 40-50 mJ pulses at 248 nm (285 fs pulse duration) with 2 Hz repetition rate. That radiation can be focused to intensities greater than 1017 W/cm2 and cause the optical field ionization of lithium. The system was used in experiments on gain generation in hydrogen-like Li III. Lasing action in hydrogen-like Li III 2-1 transition to ground state (13.5 nm) has been demonstrated for the first time. Gain G = 11 cm-1 in 5-mm long plasma column, created in LiF microcapillary, was measured. The observed gain-length product was GL = 5.5. In another set of experiments an inversion population between levels n = 3 and n = 2 in hydrogen-like BV was created using a low-energy compact laser system at 1 Hz repetition rate. Gain G = 17 cm-1 at 26.2 nm was measured in 3 mm long B2O3 microcapillary, which corresponds to GL = 5.1. The entire experimental setup can be fit on a single medium size optical table. Also propagation of laser radiation through plasma, created in microcapillaries has been investigated at various experimental conditions. Real-time plasma probing with low intensity HeNe laser beam has been performed.

Laser printed glass planar lightwave circuits with integrated fiber alignment structures

NASA Astrophysics Data System (ADS)

Desmet, A.; Radosavljevic, A.; Missinne, J.; Van Thourhout, D.; Van Steenberge, G.

2018-02-01

Femtosecond laser inscription allows straightforward manufacturing of glass planar lightwave circuits such as waveguides, interferometers, directional couplers, resonators and more complex structures. Fiber alignment structures are needed to facilitate communication with the glass planar lightwave circuit. In this study, a technique is described to create optical waveguides and alignment structures in the same laser exposure step. Using an industrial ytterbium-doped 1030 nm fiber laser pulses of 400 fs were focused into glass with a 0.4 NA objective causing permanent alteration of the material. Depending on laser parameters this modification allows direct writing of waveguides or the creation of channels after exposing the irradiated volumes to an etchant such as KOH. Writing of channels and waveguides with different laser powers, frequencies, polarisations, stage translation speeds and scan densities were investigated in fused silica and borosilicate glass. Waveguides with controlled dimensions were created, as well as etched U-grooves with a diameter of 126 μm and a sidewall roughness Ra of 255 nm. Cut back measurements were performed giving a waveguide propagation loss of 1.1 dB/cm in borosilicate glass. A coupling loss of 0.7 dB was measured for a transition between the waveguide and standard single mode fiber at 1550 nm, using index matching liquid. The described technique eliminates active alignment requirements and is useful for many applications such as microfluidic sensing, PLCs, fan-out connectors for multicore fibers and quantum optical networks.

Dual-wavelength Nd:CaLnAlO4 lasers at 1.365 and 1.390 μm

NASA Astrophysics Data System (ADS)

Loiko, Pavel; Maria Serres, Josep; Mateos, Xavier; Xu, Xiaodong; Xu, Jun; Griebner, Uwe; Petrov, Valentin; Aguiló, Magdalena; Díaz, Francesc; Major, Arkady

2018-02-01

Tetragonal calcium rare-earth aluminates, CaLnAlO4, are attractive laser host crystals. The emission of Nd3+ ions at 1.3- 1.4 μm due to the 4F3/2 -> 4I13/2 transition is of interest for medicine, fiber optics, and light conversion. We report on compact Nd:CaLnAlO4 lasers using a plane-plane cavity. With an a-cut 0.8 at.% Nd:CaYAlO4 crystal diode-pumped at 802 nm, a maximum continuous-wave output power of 365 mW was achieved at 1.365 & 1.390 μm corresponding to the σ-polarization. The 4F3/2 -> 4I13/2 laser performance of the Nd:CaLnAlO4 crystals was compared to that from a monoclinic Nd:KGd(WO4)2. At the 4F3/2-> 4I11/2 transition (1.08 μm), a Nd:CaYAlO4 micro-laser generated multi-watt output (>4 W) with a slope efficiency of 39%.

Optical cascade pumping of the 7P{sub 3/2} level in cesium atoms

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kargapol'tsev, Sergei V; Velichansky, Vladimir L; Yarovitsky, Alexander V

2005-07-31

Doppler-free absorption spectra of resonance laser fields are studied upon two-stage excitation of cesium atoms according to the schemes 6S{sub 1/2{yields}}6P{sub 3/2{yields}}6D{sub 5/2} and 6S{sub 1/2{yields}}6P{sub 3/2{yields}}8S{sub 1/2}. The obtained experimental results are in qualitative agreement with the theory. In the case of weak absorption saturation, the width of resonances is mainly determined by two-photon transitions. The efficiencies of the two variants of two-stage excitation of the 7P{sub 3/2} level are compared. The possibility of fabrication of a gas laser operating on the 455-nm 7P{sub 3/2{yields}}6S{sub 1/2} transition with the optical depopulation of the lower operating level by an additionalmore » laser is discussed. (active media)« less

Cooling atomic ions with visible and infra-red light

NASA Astrophysics Data System (ADS)

Lindenfelser, F.; Marinelli, M.; Negnevitsky, V.; Ragg, S.; Home, J. P.

2017-06-01

We demonstrate the ability to load, cool and detect singly charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using dipole-allowed transitions, we combine power broadening of a quadrupole transition at 729 nm with quenching of the upper level using a dipole allowed transition at 854 nm. By observing the resulting 393 nm fluorescence we are able to perform background-free detection of the ion. We show that this system can be used to smoothly transition between the Doppler cooling and sideband cooling regimes, and verify theoretical predictions throughout this range. We achieve scattering rates which reliably allow recooling after collision events and allow ions to be loaded from a thermal atomic beam. This work is compatible with recent advances in optical waveguides, and thus opens a path in current technologies for large-scale quantum information processing. In situations where dielectric materials are placed close to trapped ions, it carries the additional advantage of using wavelengths which do not lead to significant charging, which should facilitate high rate optical interfaces between remotely held ions.

Time of flight emission spectroscopy of laser produced nickel plasma: Short-pulse and ultrafast excitations

DOE Office of Scientific and Technical Information (OSTI.GOV)

Smijesh, N.; Chandrasekharan, K.; Joshi, Jagdish C.

2014-07-07

We report the experimental investigation and comparison of the temporal features of short-pulse (7 ns) and ultrafast (100 fs) laser produced plasmas generated from a solid nickel target, expanding into a nitrogen background. When the ambient pressure is varied in a large range of 10⁻⁶Torr to 10²Torr, the plume intensity is found to increase rapidly as the pressure crosses 1 Torr. Time of flight (TOF) spectroscopy of emission from neutral nickel (Ni I) at 361.9 nm (3d⁹(²D) 4p → 3d⁹(²D) 4s transition) reveals two peaks (fast and slow species) in short-pulse excitation and a single peak in ultrafast excitation. Themore » fast and slow peaks represent recombined neutrals and un-ionized neutrals, respectively. TOF emission from singly ionized nickel (Ni II) studied using the 428.5 nm (3p⁶3d⁸(³P) 4s→ 3p⁶3d⁹ 4s) transition shows only a single peak for either excitation. Velocities of the neutral and ionic species are determined from TOF measurements carried out at different positions (i.e., at distances of 2 mm and 4 mm, respectively, from the target surface) on the plume axis. Measured velocities indicate acceleration of neutrals and ions, which is caused by the Coulomb pull of the electrons enveloping the plume front in the case of ultrafast excitation. Both Coulomb pull and laser-plasma interaction contribute to the acceleration in the case of short-pulse excitation. These investigations provide new information on the pressure dependent temporal behavior of nickel plasmas produced by short-pulse and ultrafast laser pulses, which have potential uses in applications such as pulsed laser deposition and laser-induced nanoparticle generation.« less

Ghost features in Doppler-broadened spectra of rovibrational transitions in trapped HD+ ions

NASA Astrophysics Data System (ADS)

Patra, Sayan; Koelemeij, J. C. J.

2017-02-01

Doppler broadening plays an important role in laser rovibrational spectroscopy of trapped deuterated molecular hydrogen ions (HD+), even at the millikelvin temperatures achieved through sympathetic cooling by laser-cooled beryllium ions. Recently, Biesheuvel et al. (2016) presented a theoretical lineshape model for such transitions which not only considers linestrengths and Doppler broadening, but also the finite sample size and population redistribution by blackbody radiation, which are important in view of the long storage and probe times achievable in ion traps. Here, we employ the rate equation model developed by Biesheuvel et al. to theoretically study the Doppler-broadened hyperfine structure of the (v, L) : (0, 3) → (4, 2) rovibrational transition in HD+ at 1442 nm. We observe prominent yet hitherto unrecognized ghost features in the simulated spectrum, whose positions depend on the Doppler width, transition rates, and saturation levels of the hyperfine components addressed by the laser. We explain the origin and behavior of such features, and we provide a simple quantitative guideline to assess whether ghost features may appear. As such ghost features may be common to saturated Doppler-broadened spectra of rotational and vibrational transitions in trapped ions composed of partly overlapping lines, our work illustrates the necessity to use lineshape models that take into account all the relevant physics.

Laser-induced chemiluminescence of NaMg

NASA Astrophysics Data System (ADS)

Benard, D. J.; Michels, H. H.

1982-03-01

An unstructured continuum emission around 670 nm was observed when Mg was added to an optically pumped heat pipe containing Na and K vapor, in good agreement with ab initio calculations of the NaMg potential energy curves. The corresponding excitation spectrum showed that the incident radiation was observed by NaK molecules (X → C transitions).

A simple resonance enhanced laser ionization scheme for CO via the A1Π state

NASA Astrophysics Data System (ADS)

Sun, Z. F.; von Zastrow, A. D.; Parker, D. H.

2017-07-01

We investigate the laser ionization process taking place when the CO molecule is exposed to vacuum ultraviolet (VUV) radiation resonant with the CO A1Π (v = 0) ← X1Σ+ (v = 0) transition around 154 nm, along with the ultraviolet (UV) and visible (Red) radiation used to generate VUV by four-wave difference-frequency mixing. By measuring the CO+ ion recoil and a room temperature gas spectrum, it is possible to assign the ionization process as 1 + 1' + 1'' REMPI where the one-photon steps refer to the VUV, UV, and Red radiation, respectively. Resonance enhanced ionization of rotational states around J = 12 arise due to the overlap of the fixed wavelength UV (˜250 nm) with the R band-head of a transition assigned to CO E1Π (v = 6) ← A1Π (v = 0) with a term value of 104 787.5 cm-1. The REMPI process is efficient and polarization sensitive and should be useful in a wide range of studies involving nascent CO.

Quantum calculations for one-dimensional cooling of helium

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vredenbregt, E.; Doery, M.; Bergeman, T.

1993-05-01

We report theoretical velocity distributions for sub-Doppler laser cooling of metastable He*(2{sup 3}S), calculated with the Density Matrix and Monte Carlo Wavefunction approaches. For low-field (B = 50 mG) magnetic-field induced laser cooling on the 2{sup 3}S {yields} (2{sup 3}P, J = 2) transition ({lambda} = 1083 nm), we get a narrow, sub-Doppler structure, consisting of three, {approximately}1 photon recoil wide peaks, spaced {approximately}1 recoil apart. With increasing field, this three-peak structure develops into two velocity-selective resonance (VSR) peaks, each {approximately}2 recoils wide. For the 2{sup 3}S {yields} (3{sup 3}P, J = 2) transition ({lambda} 389 nm), VSR peaks aremore » predicted to appear at low field without the third, central peak, which only develops at higher field (B = 200 mG). Additional computations deal with polarization-gradient cooling. In general, we find that for one-dimensional cooling calculations, the Density Matrix method is more efficient than the Monte Carlo Wavefunction approach. Experiments are currently under way to test the results.« less

Novel carbazole derivatives with quinoline ring: synthesis, electronic transition, and two-photon absorption three-dimensional optical data storage.

PubMed

Li, Liang; Wang, Ping; Hu, Yanlei; Lin, Geng; Wu, Yiqun; Huang, Wenhao; Zhao, Quanzhong

2015-03-15

We designed carbazole unit with an extended π conjugation by employing Vilsmeier formylation reaction and Knoevenagel condensation to facilitate the functional groups of quinoline from 3- or 3,6-position of carbazole. Two compounds doped with poly(methyl methacrylate) (PMMA) films were prepared. To explore the electronic transition properties of these compounds, one-photon absorption properties were experimentally measured and theoretically calculated by using the time-dependent density functional theory. We surveyed these films by using an 800 nm Ti:sapphire 120-fs laser with two-photon absorption (TPA) fluorescence emission properties and TPA coefficients to obtain the TPA cross sections. A three-dimensional optical data storage experiment was conducted by using a TPA photoreaction with an 800 nm-fs laser on the film to obtain a seven-layer optical data storage. The experiment proves that these carbazole derivatives are well suited for two-photon 3D optical storage, thus laying the foundation for the research of multilayer high-density and ultra-high-density optical information storage materials. Copyright © 2014 Elsevier B.V. All rights reserved.

Highly efficient saturated visible up-conversion photoluminescent Y 2 O 3 :Er 3+ microspheres pumped with a 1.55 μm laser diode

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zhao, Jinbo; Wu, Lili; Zhang, Chuanjiang

2017-01-01

Highly efficient saturation up-conversion (UC) luminescent Y2O3:Er3+ microspheres have been successfully prepared via a hydrothermal-homogeneous precipitation method. Bright visible luminescence can be clearly seen with a 1.55 mu m laser diode excitation power as low as similar to 0.03 W cm(-2). The up-conversion (UC) emission spectra indicate that the strongest red emission with a peak situated at similar to 660 nm originated from the I-4(9/2) -> I-4(15/2) transition of Er3+. The peaks situated at similar to 520 and 550 nm can be assigned to the transition from H-2(11/2)/S-4(3/2) state to the ground state of Er3+. The high efficient saturation up-conversionmore » emission is related to the highly crystalline structure. These results indicate a new way to enhance UC radiation in rare-earth ion-doped materials prepared using a hydrothermal-homogeneous precipitation method.« less

Novel 755-nm diode laser vs. conventional 755-nm scanned alexandrite laser: Side-by-side comparison pilot study for thorax and axillary hair removal.

PubMed

Paasch, Uwe; Wagner, Justinus A; Paasch, Hartmut W

2015-01-01

Alexandrite (755 nm) and diode lasers (800-810 nm) are commonly used for hair removal. The alexandrite laser technology is somewhat cumbersome whereas new diode lasers are more robust. Recently, alexandrite-like 755 nm wavelength diodes became available. To compare the efficacy, tolerability, and subject satisfaction of a 755 nm diode laser operated in conventional (HR) and non-conventional in-motion (SHR) modes with a conventional scanned alexandrite 755 nm laser for chest and axillary hair removal. A prospective, single-center, proof of principle study was designed to evaluate the safety, efficacy and handling of a 755 nm diode laser system in comparison to a standard alexandrite 755 nm scanning hair removal laser. The new 755 nm diode is suitable to be used in SHR and HR mode and has been tested for its safety, efficacy and handling in a volunteer with success. Overall, both systems showed a high efficacy in hair reduction (88.8% 755 nm diode laser vs. 77.7% 755 nm alexandrite laser). Also, during the study period, no severe adverse effects were reported. The new 755 nm diode laser is as effective and safe as the traditional 755 nm alexandrite laser. Additionally, treatment with the 755 nm diode laser with HR and SHR modes was found to be less painful.

The Effect of Intense Laser Radiation on Atomic Collisions

NASA Astrophysics Data System (ADS)

Young, Stephen Michael Radley

1991-02-01

Available from UMI in association with The British Library. Requires signed TDF. We have carried out theoretical and experimental studies into the effect of intense laser radiation on atomic collisions. The first experiment used neon. Excitation by electron impact in a gas discharge demanded a pressure of at least 0.075 Torr. Measurement of the intensity of 3^1S_0to 3^1P_1 fluorescence has been made for the case where high intensity ASE wings in the laser profile and background laser scatter are unimportant, with the laser tuned to resonance. The field intensity required to produce strong field fluorescence (exemplified by the Mollow triplet) was found to give rise to complications capable of screening the effects sought. Our theoretical model has suggested that at finite detunings, line-centre fluorescence will dominate Rayleigh scatter and omega_3 fluorescence. Our measurements provide information on the saturation of neon fluorescence but not of the variation of the intense field collision rate. Absorption of weak field 253.7 nm laser photons by ground state mercury atoms yielded a high 6 ^3P_1 population at a lower pressure of 0.02 Torr. The Mollow triplet has been observed in the self-broadened mercury system. Dressing of the upper transition (6^3P_1rightarrow 7^3S_1) by an intense laser close to 435.8 nm yielded the strong field signal. Polarisation studies were made possible by the 3-level mercury system (radiation trapping in a 2-level system would depolarise fluorescence) perturbed by argon. The studies yielded results that were explainable in terms of the selective population of Stark shifted dressed states by a detuned, weak probe field. Use has been made of the electric-dipole radiation selection rule m_{J}=0 rightarrow m_{J^' } = 0 unless J=J^' to devise a 'Stark shift collision switch'. The competition between collision and radiation induced transitions within the mercury atom has then been studied. The resonant, strong lambda 435.8 nm field was used in conjunction with the weak lambda 253.7 nm field detuned by 0 to 6 cm^ {-1}. Measurement of fluorescence intensity in two perpendicular planes of polarisation has revealed the dominant | e_1> to | e_2> excitation channel as a function of the Stark shift by way of the U.V. detuning. Competition between the channels was dependent on the generalised Rabi frequency. However, we could only monitor the relative strength of the channels and were thus unable to say that the Stark shift switched collisions off. (Abstract shortened by UMI.).

Observation and investigation of narrow optical transitions of 167Er3+ ions in femtosecond laser printed waveguides in 7LiYF4 crystal

NASA Astrophysics Data System (ADS)

Minnegaliev, M. M.; Dyakonov, I. V.; Gerasimov, K. I.; Kalinkin, A. A.; Kulik, S. P.; Moiseev, S. A.; Saygin, M. Yu; Urmancheev, R. V.

2018-04-01

We produced optical waveguides in the 167Er3+:7 LiYF4 crystal with diameters ranging from 30 to 100 μm by using the depressed-cladding approach with femtosecond laser. Stationary and coherent spectroscopy was performed on the 809 nm optical transitions between the hyperfine sublevels of 4I15/2 and 4I9/2 multiplets of 167Er3+ ions both inside and outside of waveguides. It was found that the spectra of 167Er3+ were slightly broadened and shifted inside the waveguides compared to the bulk crystal spectra. We managed to observe a two-pulse photon echo on this transition and determined phase relaxation times for each waveguide. The experimental results show that the created crystal waveguides doped by rare-earth ions can be used in optical quantum memory and integrated quantum schemes.

The Mystery of the Electronic Spectrum of Ruthenium Monophosphide

NASA Astrophysics Data System (ADS)

Adam, Allan G.; Christensen, Ryan M.; Dore, Jacob M.; Konder, Ricarda M.; Tokaryk, Dennis W.

2016-06-01

Using PH3 as a reactant gas and ruthenium as the target metal in the UNB laser ablation spectrometer, the ruthenium monophosphide molecule (RuP) has been detected. Dispersed fluorescence experiments have been performed to determine ground state vibrational frequencies and the presence of any low-lying electronic states. Rotationally resolved spectra of two vibrational bands at 577nm and 592nm have been taken; the bands have been identified as 1-0 and 0-0 bands based on isotopic shifts. Ruthenium has seven stable isotopes and rotational transitions have been observed for six of the RuP isotopologues. RuP is isoelectronic to RuN so it is expected that RuP will have a 2Σ+ ground state and low resolution spectra indicated a likely 2Σ+ - 2Σ+ electronic transition. Further investigation has led us to believe we are observing a 2Π - 2Σ+ transition but mysteriously some important rotational branches are missing. It is hoped that new data to be recorded on a second electronic system we have observed at 535nm will help shed light on this mystery.

Electronic transitions of tantalum monofluoride

NASA Astrophysics Data System (ADS)

Ng, K. F.; Zou, Wenli; Liu, Wenjian; Cheung, A. S.-C.

2017-03-01

The electronic transition spectrum of the tantalum monofluoride (TaF) molecule in the spectral region between 448 and 560 nm has been studied using the technique of laser-ablation/reaction free jet expansion and laser induced fluorescence spectroscopy. The TaF molecule was produced by reacting laser-ablated tantalum atoms with sulfur hexafluoride gas seeded in argon. Twenty-two vibrational bands with resolved rotational structure have been recorded and analyzed, which were organized into seven electronic transitions. The X3Σ-(0+) state has been identified to be the ground state and the determined equilibrium bond length, re, and vibrational frequency, ωe, are 1.8184 Å and 700.1 cm-1, respectively. The low-lying Λ-S states and Ω sub-states of TaF were also theoretically studied at the MRCISD+Q level of theory with spin-orbit coupling. The Ω = 0+ and 2 sub-states from the -3Σ and 3Φ state have been found to be the ground and the first excited states, respectively, which agrees well with our experimental determinations. This work represents the first experimental investigation of the molecular structure of the TaF molecule.

Characteristics of laser produced plasmas of hafnium and tantalum in the 1-7 nm region

NASA Astrophysics Data System (ADS)

Li, Bowen; Otsuka, Takamitsu; Sokell, Emma; Dunne, Padraig; O'Sullivan, Gerry; Hara, Hiroyuki; Arai, Goki; Tamura, Toshiki; Ono, Yuichi; Dinh, Thanh-Hung; Higashiguchi, Takeshi

2017-11-01

Soft X-ray (SXR) spectra from hafnium and tantalum laser produced plasmas were recorded in the 1-7 nm region using two Nd:YAG lasers with pulse lengths of 170 ps and 10 ns, respectively, operating at a range of power densities. The maximum focused peak power density was 2. 3 × 1014 W cm-2 for 170 ps pulses and 1. 8 × 1012 W cm-2 for 10 ns pulses, respectively. Two intense quasicontinuous intensity bands resulting from n = 4 - n = 4 and n = 4 - n = 5 unresolved transition arrays (UTAs) dominate both sets of experimental spectra. Comparison with calculations performed with the Cowan suite of atomic structure codes as well as consideration of previous experimental and theoretical results aided identification of the most prominent features in the spectra. For the 10 ns spectrum, the highest ion stage that could be identified from the n = 4 - n = 5 arrays were lower than silver-like Hf25+ and Ta26+ (which has a 4 d 104 f ground configuration) indicating that the plasma temperature attained was too low to produce ions with an outermost 4 d subshell, while for the 170 ps plasmas the presence of significantly higher stages was deduced and lines due to 4 d-5 p transitions were clearly evident. Furthermore, we show an enhancement of emission from tantalum using dual laser irradiation, and the effect of pre-pulse durations and delay times between two pulses are demonstrated.

Effect of temperature and ridge-width on the lasing characteristics of InAs/InP quantum-dash lasers: A thermal analysis view

NASA Astrophysics Data System (ADS)

Alkhazraji, E.; Khan, M. T. A.; Ragheb, A. M.; Fathallah, H.; Qureshi, K. K.; Alshebeili, S.; Khan, M. Z. M.

2018-01-01

We investigate the thermal characteristics of multi-stack chirped barrier thickness InAs/InGaAlAs/InP quantum-dash-in-a-well lasers of different ridge widths 2, 3, 4 and 15 μm. The effect of varying this geometrical parameter on the extracted thermal resistance and characteristic temperature, and their stability with temperature are examined. The results show an inverse relation of ridge-width with junction temperature with 2 μm device exhibiting the largest junction temperature buildup owing to an associated high thermal resistance of ∼45 °C/W. Under the light of this thermal analysis, lasing behavior of different ridge-width quantum-dash (Qdash) lasers with injection currents and operating temperatures, is investigated. Thermionic carrier escape and phonon-assisted tunneling are found to be the dominant carrier transport mechanisms resulting in wide thermal spread of carriers across the available transition states of the chirped active region. An emission coverage of ∼75 nm and 3 dB bandwidth of ∼55 nm is exhibited by the 2 μm device, thus possibly exploiting the inhomogeneous optical transitions to the fullest. Furthermore, successful external modulation of a single Qdash Fabry-Perot laser mode via injection locking is demonstrated with eye diagrams at bit rates of 2-12 Gbit/s incorporating various modulation schemes. These devices are being considered as potential light sources for future high-speed wavelength-division multiplexed optical communication systems.

Laser-processing of VO2 thin films synthesized by polymer-assisted-deposition

NASA Astrophysics Data System (ADS)

Breckenfeld, Eric; Kim, Heungsoo; Gorzkowski, Edward P.; Sutto, Thomas E.; Piqué, Alberto

2017-03-01

We investigate a novel route for synthesis and laser-sintering of VO2 thin films via solution-based polymer-assisted-deposition (PAD). By replacing the traditional solvent for PAD (water) with propylene glycol, we are able to control the viscosity and improve the environmental stability of the precursor. The solution stability and ability to control the viscosity makes for an ideal solution to pattern simple or complex shapes via direct-write methods. We demonstrate the potential of our precursor for printing applications by combining PAD with laser induced forward transfer (LIFT). We also demonstrate large-area film synthesis on 4 in. diameter glass wafers. By varying the annealing temperature, we identify the optimal synthesis conditions, obtaining optical transmittance changes of 60% at a 2500 nm wavelength and a two-order-of-magnitude semiconductor-to-metal transition. We go on to demonstrate two routes for improved semiconductor-to-metal characteristics. The first method uses a multi-coating process to produce denser films with large particles. The second method uses a pulsed-UV-laser sintering step in films annealed at low temperatures (<450° C) to promote particle growth and improve the semiconductor-to-metal transition. By comparing the hysteresis width and semiconductor-to-metal transition magnitude in these samples, we demonstrate that both methods yield high quality VO2 with a three-order-of-magnitude transition.

Laser radiation at various wavelengths for decompression of intervertebral disk. Experimental observations on human autopsy specimens.

PubMed

Choy, D S; Altman, P A; Case, R B; Trokel, S L

1991-06-01

The interaction of laser radiation with the nucleus pulposus from autopsy specimens of human intervertebral disks was evaluated at different wavelengths (193 nm, 488 nm & 514 nm, 1064 nm, 1318 nm, 2150 nm, 2940 nm, and 10600 nm). A significant correlation of linear least squares fit of the mass ablated as a function of incident energy was found for all lasers used except the Excimer at 193 nm. The 2940-nm Erbium:YAG laser was most efficient in terms of mass of disk ablated per joule in the limited lower range where this wavelength was observed. At higher energy levels, the CO2 laser in the pulsed mode was most efficient. However, the Nd:YAG 1064-nm and 1318-nm lasers are currently best suited for percutaneous laser disk decompression because of the availability of usable waveguides. Carbonization of tissue with the more penetrating Nd:YAG 1064-nm laser increases the efficiency of tissue ablation and makes it comparable to the Nd:YAG 1318-nm laser.

Rare earth-doped barium gallo-germanate glasses and their near-infrared luminescence properties.

PubMed

Pisarska, Joanna; Sołtys, Marta; Górny, Agata; Kochanowicz, Marcin; Zmojda, Jacek; Dorosz, Jan; Dorosz, Dominik; Sitarz, Maciej; Pisarski, Wojciech A

2018-08-05

Near-infrared luminescence properties of Nd 3+ and Ho 3+ ions in barium gallo-germanate glasses have been reported. Several spectroscopic parameters for Nd 3+ and Ho 3+ ions have been determined from the Judd-Ofelt analysis and absorption/luminescence measurements. Quite large luminescence lifetime, quantum efficiency and stimulated emission cross-section have been obtained for the main 4 F 3/2  →  4 I 11/2 (Nd 3+ ) and 5 I 7  →  5 I 8 (Ho 3+ ) laser transitions of rare earths in barium gallo-germanate glasses. It suggests that barium gallo-germanate glass is promising for near-infrared laser application at emission wavelengths 1064 nm (Nd 3+ ) and 2020 nm (Ho 3+ ). Copyright © 2018 Elsevier B.V. All rights reserved.

Nd:AlN polycrystalline ceramics: A candidate media for tunable, high energy, near IR lasers

NASA Astrophysics Data System (ADS)

Wieg, A. T.; Grossnickle, M. J.; Kodera, Y.; Gabor, N. M.; Garay, J. E.

2016-09-01

We present processing and characterization of Nd-doped aluminum nitride (Nd:AlN) polycrystalline ceramics. We compare ceramics with significant segregation of Nd to those exhibiting minimal segregation. Spatially resolved photoluminescence maps reveal a strong correlation between homogeneous Nd doping and spatially homogeneous light emission. The spectroscopically resolved light emission lines show excellent agreement with the expected Nd electronic transitions. Notably, the lines are significantly broadened, producing near IR emission (˜1077 nm) with a remarkable ˜100 nm bandwidth at room temperature. We attribute the broadened lines to a combination of effects: multiple Nd-sites, anisotropy of AlN and phonon broadening. These broadened, overlapping lines in a media with excellent thermal conductivity have potential for Nd-based, tunable lasers with high average power.

Physical analysis on laser-induced cerebral damage

NASA Astrophysics Data System (ADS)

Luo, Xiaosen; Liu, Jiangang; Tao, Chunkan; Lan, Xiufeng; Cao, Lingyan; Pan, Weimin; Shen, Zhonghua; Lu, Jian; Ni, Xiaowu

2005-01-01

Experimental investigation on cerebral damage of adult SD rats induced by 532nm CW laser was performed. Tissue heat conductive equation was set up based on two-layered structure model. Finite difference algorithm was utilized to numerically simulate the temperature distribution in the brain tissue. Allowing for tissue response to temperature variation, free boundary model was used to discuss tissue thermal coagulation formation in brain. Experimental observations show that thermal coagulation and necrosis can be caused due to laser light absorption. The result of the calculation shows that the process of the thermal coagulation of the given mode comprises two stages: fast and slow. At the first stage, necrosis domain grows fast. Then necrosis domain growth becomes slower because of the competition between the heat diffusion into the surrounding undamaged tissue and the heat dissipation caused by blood perfusion. At the center of coagulation area no neuron was observed and at the transitional zone few nervous cells were seen by microscope. The research can provide reference data for developing clinical therapy of some kind of encephalic diseases by using 532nm laser, and for making cerebral infarction models in animal experiment.

Injection locking of violet laser diodes with a 3.2 GHz offset frequency for driving Raman transitions in 43Ca+.

PubMed

Keitch, B C; Thomas, N R; Lucas, D M

2013-03-15

Two cw single-mode violet (397 nm) diode lasers are locked to a single external-cavity master diode laser by optical injection locking. A double-pass 1.6 GHz acousto-optic modulator is used to provide a 3.2 GHz offset frequency between the two slave lasers. We achieve up to 20 mW usable output in each slave beam, with as little as 25 μW of injection power at room temperature. An optical heterodyne measurement of the beat note between the two slave beams gives a linewidth of ≤10 Hz at 3.2 GHz. We also estimate the free-running linewidth of the master laser to be approximately 3 MHz by optical heterodyning with a similar device.

Optical nonlinear properties and dynamics of interband transitions in multilayer MoS2 structures under femtosecond excitation at a wavelength of 514 nm

NASA Astrophysics Data System (ADS)

Khudyakov, D. V.; Borodkin, A. A.; Mazin, D. D.; Lobach, A. S.; Vartapetov, S. K.

2018-02-01

The optical nonlinear absorption and bleaching of aqueous suspensions of multilayer MoS2 sheets (structural modification 2H) under excitation by a 400-fs pulse at a wavelength of 514 nm is investigated using longitudinal scanning. The sample exhibits nonlinear absorption at intensities up to 15 GW cm-2, while a further increase in intensity to 70 GW cm-2 causes nonlinear bleaching with a relative change in transmission to 14%. The dynamics of interband transitions in the picosecond range is studied by femtosecond laser photolysis. The relaxation time of photoexcited excitons is measured to be 20 ± 2 ps. The transition dynamics is calculated in the three-level approximation, and the absorption cross sections of photoinduced electron transitions from the valence band to the conduction band and from the first to the second conduction band are estimated. It is shown that the optical nonlinear properties of suspensions of multilayer 2H MoS2 sheets are mainly determined by the dynamics of single-photon interband transitions.

Raman scattering and red fluorescence in the photochemical transformation of dry tryptophan particles

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lai, Chih Wei; Schwab, Mark; Hill, Steven C.

Tryptophan is a fluorescent amino acid common in proteins. Its absorption is largest for wavelengths λ ≲ 290 nm and its fluorescence emissions peak around 300–350 nm, depending upon the local environment. Here we report the observation of red fluorescence near 600 nm emerging from 488-nm continuous-wave (CW) laser photoexcitation of dry tryptophan (Trp) particles. With an excitation intensity below 0.5 kW/cm 2, dry Trp particles yield distinctive Raman scattering peaks in the presence of relatively weak and spectrally broad emissions with λ ~500–700 nm, allowing estimation of particle temperature at low excitation intensities. When the photoexcitation intensity is increasedmore » to 1 kW/cm 2 or more for a few minutes, fluorescence intensity dramatically increases by more than two orders of magnitude. The fluorescence continues to increase in intensity and gradually shift to the red when photoexcitation intensity and the duration of exposure are increased. The resulting products absorb at visible wavelengths and generate red fluorescence with λ ~ 650–800 nm with 633-nm CW laser excitation. In conclusion, we attribute the emergence of orange and red fluorescence in the Trp products to a photochemical transformation that is instigated by weak optical transitions to triplet states in Trp with 488-nm excitation and which may be expedited by a photothermal effect.« less

Raman scattering and red fluorescence in the photochemical transformation of dry tryptophan particles

DOE PAGES

Lai, Chih Wei; Schwab, Mark; Hill, Steven C.; ...

2016-05-19

Tryptophan is a fluorescent amino acid common in proteins. Its absorption is largest for wavelengths λ ≲ 290 nm and its fluorescence emissions peak around 300–350 nm, depending upon the local environment. Here we report the observation of red fluorescence near 600 nm emerging from 488-nm continuous-wave (CW) laser photoexcitation of dry tryptophan (Trp) particles. With an excitation intensity below 0.5 kW/cm 2, dry Trp particles yield distinctive Raman scattering peaks in the presence of relatively weak and spectrally broad emissions with λ ~500–700 nm, allowing estimation of particle temperature at low excitation intensities. When the photoexcitation intensity is increasedmore » to 1 kW/cm 2 or more for a few minutes, fluorescence intensity dramatically increases by more than two orders of magnitude. The fluorescence continues to increase in intensity and gradually shift to the red when photoexcitation intensity and the duration of exposure are increased. The resulting products absorb at visible wavelengths and generate red fluorescence with λ ~ 650–800 nm with 633-nm CW laser excitation. In conclusion, we attribute the emergence of orange and red fluorescence in the Trp products to a photochemical transformation that is instigated by weak optical transitions to triplet states in Trp with 488-nm excitation and which may be expedited by a photothermal effect.« less

Raman scattering and red fluorescence in the photochemical transformation of dry tryptophan particles.

PubMed

Lai, Chih Wei; Schwab, Mark; Hill, Steven C; Santarpia, Joshua; Pan, Yong-Le

2016-05-30

Tryptophan is a fluorescent amino acid common in proteins. Its absorption is largest for wavelengths λ ≲ 290 nm and its fluorescence emissions peak around 300-350 nm, depending upon the local environment. Here we report the observation of red fluorescence near 600 nm emerging from 488-nm continuous-wave (CW) laser photoexcitation of dry tryptophan (Trp) particles. With an excitation intensity below 0.5 kW/cm², dry Trp particles yield distinctive Raman scattering peaks in the presence of relatively weak and spectrally broad emissions with λ ∼500-700 nm, allowing estimation of particle temperature at low excitation intensities. When the photoexcitation intensity is increased to 1 kW/cm² or more for a few minutes, fluorescence intensity dramatically increases by more than two orders of magnitude. The fluorescence continues to increase in intensity and gradually shift to the red when photoexcitation intensity and the duration of exposure are increased. The resulting products absorb at visible wavelengths and generate red fluorescence with λ ∼ 650-800 nm with 633-nm CW laser excitation. We attribute the emergence of orange and red fluorescence in the Trp products to a photochemical transformation that is instigated by weak optical transitions to triplet states in Trp with 488-nm excitation and which may be expedited by a photothermal effect.

Experimental Results from a Laser-Triggered, Gas-Insulated, Spark-Gap Switch

NASA Astrophysics Data System (ADS)

Camacho, J. F.; Ruden, E. L.; Domonkos, M. T.

2017-10-01

We are performing experiments on a laser-triggered spark-gap switch with the goal of studying the transition from photoionization to current conduction. The discharge of current through the switch is triggered by a focused 532-nm wavelength beam from a Q-switched Nd:YAG laser with a pulse duration of about 10 ns. The trigger pulse is delivered along the longitudinal axis of the switch, and the focal spot can be placed anywhere along the axis of the 5-mm, gas-insulated gap between the switch electrodes. The switch test bed is designed to support a variety of working gases (e.g., Ar, N2) over a range of pressures. Electrical and optical diagnostics are used to measure switch performance as a function of parameters such as charge voltage, trigger pulse energy, insulating gas pressure, and gas species. A Mach-Zehnder imaging interferometer system operating at 532 nm is being used to obtain interferograms of the discharge plasma in the switch. We are also developing a 1064-nm interferometry diagnostic in an attempt to measure plasma free electron and neutral gas density profiles simultaneously within the switch gap. Results from our most recent experiments will be presented.

Relative quantum yield of I-asterisk(2P1/2) in the tunable laser UV photodissociation of i-C3F7I and n-C3F7I - Effect of temperature and exciplex emission

NASA Technical Reports Server (NTRS)

Smedley, J. E.; Leone, S. R.

1983-01-01

Wavelength-specific relative quantum yields of metastable I from pulsed laser photodissociation of i-C3F7I and n-C3F7I in the range 265-336 nm are determined by measuring the time-resolved infrared emission from the atomic I(P-2(1/2) P-2(3/2) transition. It is shown that although this yield appears to be unity from 265 to 298 nm, it decreases dramatically at longer wavelengths. Values are also reported for the enhancement of emission from metastable I due to exciplex formation at several temperatures. The exciplex formation emission increases linearly with parent gas pressure, but decreases with increasing temperature. Absorption spectra of i- and n-C3F7I between 303 and 497 K are presented, and the effect of temperature on the quantum yields at selected wavelengths greater than 300 nm, where increasing the temperature enhances the absorption considerably, are given. The results are discussed in regard to the development of solar-pumped iodine lasers.

The influence of UV laser radiation on the absorption and luminescence of photothermorefractive glasses containing silver ions

NASA Astrophysics Data System (ADS)

Ignat'ev, A. I.; Ignat'ev, D. A.; Nikonorov, N. V.; Sidorov, A. I.

2015-08-01

It is experimentally shown that irradiation of silver-containing glasses by nanosecond laser pulses with a wavelength of 248 nm leads to the formation of unstable point defects (having absorption bands in the UV and visible spectral ranges) in the irradiated region and causes the transition of ions and charged molecular silver clusters to the neutral state, which is accompanied by an increase in the luminescence intensity in the visible spectral range. The influence of pulsed laser irradiation is compared with the effect of exposure to cw UV light of a mercury lamp. Some models are proposed to explain the influence of the laser effect on the optical properties of glasses.

Fine wavelength control in 1.3 μm Nd:YAG lasers by electro-optical crystal lens

NASA Astrophysics Data System (ADS)

Lü, Yanfei; Zhang, Jing; Liu, Huilong; Xia, Jing; Fu, Xihong; Zhang, Anfeng

2014-02-01

A diode-pumped tunable and multi-wavelength continuous-wave Nd:YAG laser based on the 4F3/2-4I13/2 transition has been demonstrated for the first time. The combination of the glass plane positioned at the Brewster angle and the electro-optical crystal KH2PO4 (KDP) lens formed a Lyot filter in the cavity and compressed the available gain bandwidth. With an adjustable voltage applied to the KDP crystal lens, the laser wavelength could be tuned from 1333.8 to 1338.2 nm. Moreover, we can also realize cw dual-wavelength and triple-wavelength lasers with smaller wavelength separation by adjusting the free spectral range of the Lyot filter.

Impact of oxygen chemistry on the emission and fluorescence spectroscopy of laser ablation plumes

NASA Astrophysics Data System (ADS)

Hartig, K. C.; Brumfield, B. E.; Phillips, M. C.; Harilal, S. S.

2017-09-01

Oxygen present in the ambient gas medium may affect both laser-induced breakdown spectroscopy (LIBS) and laser-induced fluorescence (LIF) emission through a reduction of emission intensity and persistence. In this study, an evaluation is made on the role of oxygen in the ambient environment under atmospheric pressure conditions in LIBS and laser ablation (LA)-LIF emission. To generate plasmas, 1064 nm, 10 ns pulses were focused on an aluminum alloy sample. LIF was performed by frequency scanning a CW laser over the 396.15 nm (3s24s 2S1/2 → 3s23p 2P°3/2) Al I transition. Time-resolved emission and fluorescence signals were recorded to evaluate the variation in emission intensity caused by the presence of oxygen. The oxygen partial pressure (po) in the atmospheric pressure environment using N2 as the makeup gas was varied from 0 to 400 Torr O2. 2D-fluorescence spectroscopy images were obtained for various oxygen concentrations for simultaneous evaluation of the emission and excitation spectral features. Results showed that the presence of oxygen in the ambient environment reduces the persistence of the LIBS and LIF emission through an oxidation process that depletes the density of atomic species within the resulting laser-produced plasma (LPP) plume.

Er3+-Tm3+-Yb3+:CaMoO4 phosphor as an outstanding upconversion-based optical temperature sensor and optical heater.

PubMed

Dey, Riya; Kumar Rai, Vineet

2017-03-22

Optical temperature sensing in Er 3+ -Tm 3+ -Yb 3+ codoped CaMoO 4 phosphor prepared by chemical co-precipitation route based on the near infrared (NIR) to green upconversion emission from Er 3+ ion is reported. The variation with respect to external temperature in emission intensity ratio of the green emissions around 530 nm and 552 nm, corresponding to the 2 H 11/2  →  4 I 15/2 and 4 S 3/2  →  4 I 15/2 transitions respectively, under 980 nm excitation has been studied in detail, to report the sensing property of the prepared material; the maximum sensor sensitivity ∼0.0182 K -1 was attained at 413 K. The laser induced optical heating within the prepared phosphor has been explored and the heat generation caused by the laser effect has been verified by comparison of experimental and calculated data.

Continuous-wave modulation of a femtosecond oscillator using coherent molecules.

PubMed

Gold, D C; Karpel, J T; Mueller, E A; Yavuz, D D

2018-03-01

We describe a new method to broaden the frequency spectrum of a femtosecond oscillator in the continuous-wave (CW) domain. The method relies on modulating the femtosecond laser using four-wave mixing inside a Raman-based optical modulator. We prepare the modulator by placing deuterium molecules inside a high-finesse cavity and driving their fundamental vibrational transition using intense pump and Stokes lasers that are locked to the cavity modes. With the molecules prepared, any laser within the optical region of the spectrum can pass through the system and be modulated in a single pass. This constitutes a CW optical modulator at a frequency of 90 THz with a steady-state single-pass efficiency of ∼10 -6 and transient (10 μs-time-scale) single-pass efficiency of ∼10 -4 . Using our modulator, we broaden the initial Ti:sapphire spectrum centered at 800 nm and produce upshifted and downshifted sidebands centered at wavelengths of 650 nm and 1.04 μm, respectively.

Resonance-enhanced two-photon excitation of CaI

NASA Astrophysics Data System (ADS)

Casero-Junquera, Elena; Lawruszczuk, Rafal; Rostas, Joëlle; Taieb, Guy

1994-07-01

Induced fluorescence following visible (620-655 nm) laser excitation of the CaI radical has been detected not only in the same region (B, A-X transitions), but also in the UV (315-330 nm). The UV two-photon excitation spectrum consists of narrow bands appearing at laser frequencies located within certain bands of the Δ v = 1, 0 sequences of the B 2Σ +-X 2Σ + and A 2Π 1/2-X 2Σ + systems. The main peaks are tentatively assigned to resonance-enhanced excitation of a single vibrational level of the lowest Rydberg D 2Σ + state from successive vibrational levels of the ground state. The excitation process is a one-color two-photon optical—optical-double-resonance via B 2Σ + and A 2Π 1/2 intermediate levels. This analysis is supported by the absorption spectrum observed long ago by Walters and Barratt. The absorption and laser excitation complementary data have been used to derive approximate molecular constants for the D state.

Trapped-Ion Quantum Simulation of an Ising Model with Transverse and Longitudinal Fields

DTIC Science & Technology

2013-03-29

resonant λ = 355 nm laser beams which drive stimulated Raman transitions [33, 34]. The beams intersect at right angles so that their wavevector difference...ated by a pair of Raman laser beams with a beatnote frequency of ωS , with the field amplitude determined by the beam intensities. The field directions...cool- ing, followed by optical pumping to the state |↓↓↓ ..〉z and 100 µs of Raman sideband cooling that prepares the motion of all modes along ∆~k in

Effect of concentration variation on 2.0 µm emission of Ho3+-doped SiO2-Al2O3-Na2CO3-SrF2-CaF2 oxyfluorosilicate glasses

NASA Astrophysics Data System (ADS)

Gelija, Devarajulu; Borelli, Deva Prasad Raju

2018-02-01

The concentration variation of Ho3+ ion-doped SiO2-Al2O3-Na2CO3-SrF2-CaF2 glasses has been prepared by conventional melt quenching method. The thermal stability of 1 mol % of Ho3+-doped oxyfluorosilicate glass has been calculated using the differential thermal analysis (DTA) spectra. The phenomenological Judd-Ofelt intensity parameters Ωλ ( λ = 2, 4 and 6) were calculated for all concentrations of Ho3+ ions. The luminescence spectra in visible region of Ho3+ ion-doped glasses were recorded under the excitation wavelength of 452 nm. The spectra consists of several intense emission bands (5F4, 5S2) → 5I8 (547 nm), 5F3 → 5I8 (647 nm), 5F5 → 5I7 (660 nm) and (5F4, 5S2) → 5I7 (750 nm) in the range 500-780 nm. The fluorescence emission at ˜2.0 µm (5I7 → 5I8) was observed under the excitation of 488 nm Ar-ion laser. The stimulated emission cross section for 5I7 → 5I8 transition (˜2.0 µm) varies from 8.46 to 9.52 × 10-21 cm2, as calculated by the Fuchtbauer-Ladenburg (FL) theory. However, Mc-Cumber theory was used to calculate emission cross section values about 4.24-5.75 × 10-21 cm2 for the 5I7 → 5I8 transition in all concentrations of Ho3+-doped oxyfluorosilicate glasses. Therefore, these results reveal that the 0.5 mol % of Ho3+-doped oxyfluorosilicate glasses, exhibiting higher emission cross section, has potentially been used for laser applications at ˜ 2.0 µm.

Comparison of the ablation ability of nucleus pulposus after 1,064 nm Nd:YAG laser and 980 nm diode laser radiation.

PubMed

Yin, Jian; Han, Zhengfeng; Guo, Baofeng; Guo, Han; Zhang, Tongtong; Zeng, Yanjun; Ren, Longxi

2015-07-01

To compare the ablation ability of nucleus pulposus after 1,064 nm Nd:YAG laser and 980 nm diode laser radiation. Goat spine specimen (GSS) was radiated using Nd:YAG laser and 980 nm diode laser and then divided into five groups based on the final energy--200, 400, 600, 800 and 1,000 J groups. The ablation quality of nucleus pulposus after radiation was recorded. The ablation quality of GSS was greater at higher radiation energies in both lasers. When compared at the same energy level, the ablation quality of GSS was greater in 980 nm diode laser than in 1,064 nm Nd:YAG laser. Statistical significance was observed in 200 and 400 J groups (P < 0.05) and in 600, 800 and 1,000 J groups (P < 0.01). Radiation with 980 nm diode laser showed better ablation ability than 1,064 nm Nd:YAG laser.

ARPA solid state laser and nonlinear materials program

NASA Astrophysics Data System (ADS)

Moulton, Peter F.

1994-06-01

The Research Division of Schwartz Electro-Optics, as part of the ARPA Solid State Laser and Nonlinear Materials Program, conducted a three-year study 'Erbium-Laser-Based Infrared Sources.' The aim of the study was to improve the understanding of semiconductor-laser-pumped, infrared (IR) solid state lasers based on the trivalent rare-earth ion erbium (Er) doped into a variety of host crystals. The initial program plan emphasized operation of erbium-doped materials on the 2.8-3.0 micrometers laser transition. Pulsed, Q-switched sources using that transition, when employed as a pump source for parametric oscillators, can provide tunable mid-IR energy. The dynamics of erbium lasers are more complex than conventional neodymium (Nd)-doped lasers and we intended to use pump-probe techniques to measure the level and temporal behavior of gain in various materials. To do so we constructed a number of different cw Er-doped lasers as probe sources and employed the Cr:LiSAF(LiSrAlF6) laser as a pulsed pump source that would simulate pulsed diode arrays. We identified the 970-nm wavelength pump band of Er as the most efficient and were able to make use of recently developed cw and pulsed InGaAs strained-quantum-well diode lasers in the effort. At the conclusion of the program we demonstrated the first pulsed diode bar pumping of the most promising materials for pulsed operation, the oxide garnets YSGG and GGG and the fluoride BaY2F8.

Spectroscopic analysis of a novel Nd3+-activated barium borate glass for broadband laser amplification

NASA Astrophysics Data System (ADS)

Vázquez, G. V.; Muñoz H., G.; Camarillo, I.; Falcony, C.; Caldiño, U.; Lira, A.

2015-08-01

Spectroscopic parameters of a novel Nd3+-activated barium borate (BBONd) glass have been analyzed for broadband laser amplification. The Judd-Ofelt (JO) intensity parameters were determined through a systematic analysis of the absorption spectrum of Nd3+ ions in the BBONd glass. High values of the JO intensity parameters reveal a great centro-symmetrical loss of the Nd3+ sites and high covalency degree of the ligand field. The very high Ω6 intensity parameter value makes evident both a great structural distortion of the Nd3+ sites and a strong electron-phonon coupling between Nd3+ and free OH- ions, which is consistent with the phonon energy maximum (3442.1 cm-1) recorded by Raman spectroscopy. This strong electron-phonon coupling favors high effective bandwidth and gain bandwidth values of the laser emission (4F3/2 → 4I11/2) of Nd3+ ions. The electric-dipole oscillator strengths of all the Nd3+ absorption transitions, and in particular that of the hypersensitive transition (4I9/2 → 4G5/2), are enhanced by this great structural distortion of the host. Broadband laser amplification of the 4F3/2 → 4I11/2 emission (1062 nm) of Nd3+ ions in the BBONd glass pumped at 805 nm (4I9/2 → 4F5/2 + 2H9/2) is evaluated through the main fluorescent parameters in competition with non-radiative processes. In general, the BBONd glass exhibits spectroscopic parameters comparable with those reported in the literature for broadband laser amplification into the IR region.

Nanoparticle formation after nanosecond-laser irradiation of thin gold films

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ratautas, Karolis; Gedvilas, Mindaugas; Raciukaitis, Gediminas

2012-07-01

Evolution in nanoparticle formation was observed after nanosecond-laser irradiation of thin gold films on a silicon substrate and physical phenomena leading to the formation of nanoparticles were studied. Gold films of different thickness (3, 5, 10, 15, 20, and 25 nm) were evaporated on the silicon (110) substrate and irradiated with the pulsed nanosecond laser using different pulse energies and the number of pulses in a burst. Experimentally morphological changes appeared in the films only when the pulse energy was high enough to initiate the phase transition. The threshold energy density for phase transitions in the films was estimated frommore » the thermal model of the laser beam and sample interaction. With the pulse energy just above the threshold, it was possible to observe evolution of nanoparticle formation from a plane metal film by changing the number of pulses applied, as duration of the pulse burst represented the time how long the liquid phase existed. The final size of nanoparticles was a function of the film thickness and was found to be independent of the pulse energy and the number of pulses.« less

Iodine Tagging Velocimetry in a Mach 10 Wake

NASA Technical Reports Server (NTRS)

Balla, Robert Jeffrey

2013-01-01

A variation on molecular tagging velocimetry (MTV) [1] designated iodine tagging velocimetry (ITV) is demonstrated. Molecular iodine is tagged by two-photon absorption using an Argon Fluoride (ArF) excimer laser. A single camera measures fluid displacement using atomic iodine emission at 206 nm. Two examples ofMTVfor cold-flowmeasurements areN2OMTV [2] and Femtosecond Laser Electronic Excitation Tagging [3]. These, like most MTV methods, are designed for atmospheric pressure applications. Neither can be implemented at the low pressures (0.1- 1 Torr) in typical hypersonic wakes. Of all the single-laser/singlecamera MTV approaches, only Nitric-Oxide Planar Laser Induced Fluorescence-based MTV [4] has been successfully demonstrated in a Mach 10 wake. Oxygen quenching limits transit times to 500 ns and accuracy to typically 30%. The present note describes the photophysics of the ITV method. Off-body velocimetry along a line is demonstrated in the aerothermodynamically important and experimentally challenging region of a hypersonic low-pressure near-wake in a Mach 10 air wind tunnel. Transit times up to 10 µs are demonstrated with conservative errors of 10%.

Pressure shift coefficient measurements in an RF discharge for Ar 4s[3/2]2—5p[3/2]3 transition with the help of diodelaser absorption spectroscopy

NASA Astrophysics Data System (ADS)

Chernyshov, A. K.; Mikheyev, P. A.; Lunev, N. N.; Azyazov, V. N.

2018-04-01

Optically pumped all-rare-gas laser (OPRGL) with unique properties were recently proposed with a possibility to obtain the laser power on the order of hundreds of Watts from a cubic centimeter. To provide high laser efficiency, the pumping radiation has to match the absorption spectrum of the rare gas metastables. To meet this condition a reliable diagnostics of the key parameters of the active medium is required and knowledge of the broadening and shift coefficients for corresponding transitions of rare gases is necessary. In this paper, the diode-laser absorption spectroscopy was employed to determine the pressure shift coefficient for 811.5 nm Ar line. The value of obtained coefficient in pure argon reduced to 300 K is -(2.1 ± 0.1) × 10-10 s-1cm3. In the course of the study the pressure broadening coefficient was also evaluated and found to be (2.4 ± 0.5) × 10-10 s-1cm3.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Trickl, T.; Kung, A. H.; Lee, Y. T.

Measurements of several transitions in krypton carried out with a high-resolution extreme ultraviolet (xuv) laser source in 1987 were recently reanalyzed. This analysis, based on simulating the Doppler-broadened line shape of the iodine reference lines with new, greatly improved iodine reference data, yielded an order-of-magnitude improvement in the agreement between several {sup 86}Kr transition frequencies between 94.5 nm and 116.5 nm to {+-}5x10{sup -9}. The overall relative uncertainty is estimated to be {+-}6x10{sup -9}, which matches the best accuracies achieved in nanosecond short-wavelength experiments. The influence of frequency chirping in the pulsed dye amplifier chain was estimated to be rathermore » low and to vary approximately between -7.1 MHz and +5.0 MHz for the three laser dyes used in this experiment. It is concluded that with an even more careful laser design the chirp-induced frequency shifts could be reduced to less than 1 MHz. Based on the analysis of the presumable chirp effects a correction for the {sup 86}Kr atlas by Kaufman and Humphries -0.055 53 cm{sup -1} is determined, which agrees with the result of a very recent two-photon experiment with frequency combs within just 0.000 46 cm{sup -1} (14 MHz), i.e., well within the combined errors of the three data sources involved in the intercomparison.« less

Three-photon excitation of 2,5-bis(4-biphenyl)oxazole: steady-state and time-resolved intensities and anisotropies

NASA Astrophysics Data System (ADS)

Gryczynski, Ignacy; Malak, Henryk; Hell, Stefan W.; Lakowicz, Joseph R.

1996-10-01

Three-photon excitation of 2,5-bis(4-biphenyl) oxazole (BBO) was observed when it was excited with the fundamental output of a femtosecond Ti:sapphire laser above 820 nm. The emission spectrum of BBO was identical for one-, two-, and three-photon excitation at 320, 640, and 960 nm, respectively. In toluene and triacetin, the emission intensity of BBO depended on the square of the laser power for wavelengths below 820 nm and displayed a sharp transition to a cubic dependence at longer wavelengths. The spatial distribution of the emission of BBO with three- photon excitation was more strongly localized than for two- photon excitation of a coumarin fluorophore at the same wavelength. The same single exponential intensity decay was observed for one-, two-, and three-photon excitation. However, the frequency domain anisotropy decay with three- photon excitation at 960 nm revealed a larger time-zero anisotropy, larger differential polarized phase angle, and larger modulated anisotropy than is possible for two-photon excitation with colinear oscillators. In triacetin, the anisotropy is not constant for three-photon excitation at different wavelengths. Surprisingly, the fluorescence intensities for three-photon excitation were only about 100- fold less than for two-photon excitation. The increasing availability of Ti:sapphire lasers suggests that multiphoton excitation can become a common tool in fluorescence spectroscopy.

Development of ytterbium-doped oxyfluoride glasses for laser cooling applications.

PubMed

Krishnaiah, Kummara Venkata; de Lima Filho, Elton Soares; Ledemi, Yannick; Nemova, Galina; Messaddeq, Younes; Kashyap, Raman

2016-02-26

Oxyfluoride glasses doped with 2, 5, 8, 12, 16 and 20 mol% of ytterbium (Yb(3+)) ions have been prepared by the conventional melt-quenching technique. Their optical, thermal and thermo-mechanical properties were characterized. Luminescence intensity at 1020 nm under laser excitation at 920 nm decreases with increasing Yb(3+) concentration, suggesting a decrease in the photoluminescence quantum yield (PLQY). The PLQY of the samples was measured with an integrating sphere using an absolute method. The highest PLQY was found to be 0.99(11) for the 2 mol% Yb(3+): glass and decreases with increasing Yb(3+) concentration. The mean fluorescence wavelength and background absorption of the samples were also evaluated. Upconversion luminescence under 975 nm laser excitation was observed and attributed to the presence of Tm(3+) and Er(3+) ions which exist as impurity traces with YbF3 starting powder. Decay curves for the Yb(3+): (2)F5/2 → (2)F7/2 transition exhibit single exponential behavior for all the samples, although lifetime decrease was observed for the excited level of Yb(3+) with increasing Yb(3+) concentration. Also observed are an increase in the PLQY and a slight decrease in lifetime with increasing the pump power. Finally, the potential of these oxyfluoride glasses with high PLQY and low background absorption for laser cooling applications is discussed.

Development of ytterbium-doped oxyfluoride glasses for laser cooling applications

PubMed Central

Krishnaiah, Kummara Venkata; Soares de Lima Filho, Elton; Ledemi, Yannick; Nemova, Galina; Messaddeq, Younes; Kashyap, Raman

2016-01-01

Oxyfluoride glasses doped with 2, 5, 8, 12, 16 and 20 mol% of ytterbium (Yb3+) ions have been prepared by the conventional melt-quenching technique. Their optical, thermal and thermo-mechanical properties were characterized. Luminescence intensity at 1020 nm under laser excitation at 920 nm decreases with increasing Yb3+ concentration, suggesting a decrease in the photoluminescence quantum yield (PLQY). The PLQY of the samples was measured with an integrating sphere using an absolute method. The highest PLQY was found to be 0.99(11) for the 2 mol% Yb3+: glass and decreases with increasing Yb3+ concentration. The mean fluorescence wavelength and background absorption of the samples were also evaluated. Upconversion luminescence under 975 nm laser excitation was observed and attributed to the presence of Tm3+ and Er3+ ions which exist as impurity traces with YbF3 starting powder. Decay curves for the Yb3+: 2F5/2 → 2F7/2 transition exhibit single exponential behavior for all the samples, although lifetime decrease was observed for the excited level of Yb3+ with increasing Yb3+ concentration. Also observed are an increase in the PLQY and a slight decrease in lifetime with increasing the pump power. Finally, the potential of these oxyfluoride glasses with high PLQY and low background absorption for laser cooling applications is discussed. PMID:26915817

Studies on nanosecond 532nm and 355nm and ultrafast 515nm and 532nm laser cutting super-hard materials

NASA Astrophysics Data System (ADS)

Zhang, Jie; Tao, Sha; Wang, Brian; Zhao, Jay

2017-02-01

In this paper, micro-processing of three kinds of super-hard materials of poly-crystal diamond (PCD)/tungsten-carbide (WC), CVD-diamond and cubic boron nitride (CNB) has been systematically studied using nanosecond laser (532nm and 355nm), and ultrafast laser (532nm and 515nm). Our purpose is to investigate a full laser micro-cutting solution to achieve a ready-to-use cutting tool insert (CTI). The results show a clean cut with little burns and recasting at edge. The cutting speed of 2-10mm/min depending on thickness was obtained. The laser ablation process was also studied by varying laser parameters (wavelength, pulse width, pulse energy, repetition rate) and tool path to improve cutting speed. Also, studies on material removal efficiency (MRE) of PCD/WC with 355nm-ns and 515nm-fs laser as a function of laser fluence show that 355nm-ns laser is able to achieve higher MRE for PCD and WC. Thus, ultrafast laser is not necessarily used for superhard material cutting. Instead, post-polishing with ultrafast laser can be used to clean cutting surface and improve smoothness.

The effect of ultrafast laser wavelength on ablation properties and implications on sample introduction in inductively coupled plasma mass spectrometry

PubMed Central

LaHaye, N. L.; Harilal, S. S.; Diwakar, P. K.; Hassanein, A.; Kulkarni, P.

2015-01-01

We investigated the role of femtosecond (fs) laser wavelength on laser ablation (LA) and its relation to laser generated aerosol counts and particle distribution, inductively coupled plasma-mass spectrometry (ICP-MS) signal intensity, detection limits, and elemental fractionation. Four different NIST standard reference materials (610, 613, 615, and 616) were ablated using 400 nm and 800 nm fs laser pulses to study the effect of wavelength on laser ablation rate, accuracy, precision, and fractionation. Our results show that the detection limits are lower for 400 nm laser excitation than 800 nm laser excitation at lower laser energies but approximately equal at higher energies. Ablation threshold was also found to be lower for 400 nm than 800 nm laser excitation. Particle size distributions are very similar for 400 nm and 800 nm wavelengths; however, they differ significantly in counts at similar laser fluence levels. This study concludes that 400 nm LA is more beneficial for sample introduction in ICP-MS, particularly when lower laser energies are to be used for ablation. PMID:26640294

Study of visible luminescence spectra from Nd3+ doped TPO glass upon 808 nm excitation

NASA Astrophysics Data System (ADS)

Azam, Mohd; Rai, Vineet Kumar

2018-05-01

The Nd3+ doped TPO glasses have been prepared by melting and quenching method using the high temperature electric furnace. The upconversion (UC) spectra of Nd3+ doped TPO glasses at different concentration of rare ions have been recorded in the 400-700 nm wavelength range upon 808 nm laser excitation source. In the UC emission process, there are four bands centered at ˜495 nm, 546 nm, 602 nm and 653 nm respectively in the visible range were observed. But the green and red bands centered at˜546 nm and ˜653 nm corresponding to the 4G7/2 → 4I9/2 and 4G7/2 → 4I13/2 transitions respectively have been observed as the strong bands. The UC emission mechanism was observed as two photon process. The material can be used as a good NIR to visible upconverter and non-colour tunable display.

Theoretical modeling of diode-laser-pumped 3-μm Er3+ crystal lasers

NASA Astrophysics Data System (ADS)

Tikerpae, Mark; Jackson, Stuart D.; King, Terence A.

1997-05-01

We present results from a theoretical model that has been developed to simulate the 3-micrometer laser transition in Er3+ doped Y3Al5O12 (YAG), Y2Sc2Ga3O12 (YSGG), LiYF4 (YLF) and BaY2F8 (BaYF) host crystals. The rate equations for the lowest seven energy levels of Er3+ were solved numerically and laser action was simulated under cw, gain-switched (pulse pumped) and Q-switched operation with optical pumping at wavelengths of 975 nm and 795 nm. The relative performance of each laser crystal was compared under identical pumping and cavity conditions to establish the optimum crystal host, doping concentration and pump wavelength for each mode of operation. Some unexpected saturation effects were investigated that could limit the maximum practical pump fluence used for high energy Q-switched systems. We investigate possible additional multi-ion energy transfer processes that may cause the decrease in efficiency that is observed experimentally at high Er3+ ion concentrations. In addition, lower laser level deactivation by co-doping with Pr3+ in BaYF was simulated and compared with singly doped Er:BaYF for a range of Er3+ and Pr3+ concentrations. It was found that co-doping was not as effective as the cooperative upconversion process present in singly doped Er3+ crystals for efficient laser operation.

Interface modification based ultrashort laser microwelding between SiC and fused silica.

PubMed

Zhang, Guodong; Bai, Jing; Zhao, Wei; Zhou, Kaiming; Cheng, Guanghua

2017-02-06

It is a big challenge to weld two materials with large differences in coefficients of thermal expansion and melting points. Here we report that the welding between fused silica (softening point, 1720°C) and SiC wafer (melting point, 3100°C) is achieved with a near infrared femtosecond laser at 800 nm. Elements are observed to have a spatial distribution gradient within the cross section of welding line, revealing that mixing and inter-diffusion of substances have occurred during laser irradiation. This is attributed to the femtosecond laser induced local phase transition and volume expansion. Through optimizing the welding parameters, pulse energy and interval of the welding lines, a shear joining strength as high as 15.1 MPa is achieved. In addition, the influence mechanism of the laser ablation on welding quality of the sample without pre-optical contact is carefully studied by measuring the laser induced interface modification.

2  μm laser oscillation of Ho3+:Tm3+-codoped silica microspheres.

PubMed

Peng, Longxiang; Huang, Yantang; Duan, Yafan; Zhuang, Shijian; Liao, Tingdi; Xu, Canhua

2017-09-10

2 μm laser oscillation with a low threshold has been achieved in Ho 3+ :Tm 3+ -codoped silica microspheres (HTCSMs). Ho 3+ :Tm 3+ -codoped solgel functionalization film is applied to the surface of a silica microsphere, and an optical tapered fiber is adopted to couple an 808 nm continuous-wave laser to serve as the pump light source. Multimode and single-mode laser oscillations around 2 μm within the eye-safe wave band are observed due to the I 7 5→I 8 5 transitions of Ho 3+ ions sensitized by Tm 3+ . The morphology characteristics of microspheres determine the multimode laser oscillation spectrum. The free spectral range is in good accordance with the calculated value based on Mie scattering theory. The HTCSM laser oscillation shows characteristics of good capability, simple process, high flexibility, and low cost.

Comparative study of Nd:KGW lasers pumped at 808 nm and 877 nm

NASA Astrophysics Data System (ADS)

Huang, Ke; Ge, Wen-Qi; Zhao, Tian-Zhuo; He, Jian-Guo; Feng, Chen-Yong; Fan, Zhong-Wei

2015-10-01

The laser performance and thermal analysis of Nd:KGW laser continuously pumped by 808 nm and 877 nm are comparatively investigated. Output power of 670 mW and 1587 mW, with nearly TEM00 mode, are achieved respectively at 808 nm pump and 877 nm pump. Meanwhile, a high-power passively Q-switched Nd:KGW/Cr4+:YAG laser pumped at 877 nm is demonstrated. An average output power of 1495 mW is obtained at pump power of 5.22 W while the laser is operating at repetition of 53.17 kHz. We demonstrate that 877 nm diode laser is a more potential pump source for Nd:KGW lasers.

Tunable diode laser-pumped Tm,Ho:YLF laser operated in continuous-wave and Q-switched modes

NASA Technical Reports Server (NTRS)

Mcguckin, B. T.; Hemmati, H.; Menzies, R. T.

1992-01-01

Tunable continuous-wave and pulsed laser output was obtained from a Tm-sensitized Ho:YLiF4 crystal at subambient temperatures when longitudinally pumped with a diode laser array. A conversion efficiency of 42 percent and slope efficiency of approximately 60 percent relative to the absorbed pumped power have been achieved at a crystal temperature of 275 K. The emission spectrum was etalon tunable over a range of 16/cm centered at 2067 nm with fine tuning capability of the transition frequency with crystal temperature at measured rate of -0.03/cm/K. Output energies of 0.22 mJ per pulse and 22 ns pulse duration were recorded at Q-switch frequencies that correspond to an effective upper laser level lifetime of 6 ms, and a pulse energy extraction efficiency of 64 percent.

Two-photon pumped amplified spontaneous emission based on all-inorganic perovskite nanocrystals embedded with gold nanorods

NASA Astrophysics Data System (ADS)

Liu, Shaoying; Fang, Xiaohui; Wang, Yimeng; Zhang, Xinping

2018-07-01

CsPbBr3 nanocrystals have attracted great interest owing to their high fluorescence quantum efficiency, adjustable photoluminescence wavelength, and good stability. We report a device that consists of disordered gold nanorods underneath a film of CsPbBr3 nanocrystals. Two-photon pumping using femtosecond laser pulses at 800 nm enables amplified spontaneous emission (ASE) at about 523 nm. In this work, a narrow peak with linewidth of 5 nm is observed when the pump fluence reaches a low threshold of 0.65 mJ/cm2. The results show that plasmonic resonance of gold nanorods improves the emission transition rate and enables low threshold ASE.

Nonlinear absorption and optical limiting in gold-precipitated glasses induced by a femtosecond laser

NASA Astrophysics Data System (ADS)

Qu, Shiliang; Gao, Yachen; Jiang, Xiongwei; Zeng, Huidan; Song, Yinglin; Qiu, Jianrong; Zhu, Congshan; Hirao, K.

2003-09-01

Nonlinear absorptions of Au nanoparticles precipitated silicate glasses by irradiation of a focused femtosecond pulsed laser were investigated using Z-scan technique with 8 ns pulses at 532 nm. Optical limiting (OL) effects in such glasses have been also measured. It is observed that the behaviors of transition from saturable absorption to reverse saturable absorption and the OL performances for different samples are significantly different, which depend drastically on the irradiation power density of the femtosecond laser used for the Au nanoparticles precipitation in the glass. Strong nonlinear absorptions in these samples are mainly attributed to the surface plasmon resonance (SPR) and free carrier absorptions of the precipitated Au nanoparticles.

Single- and dual-wavelength laser operation of a diode-pumped Nd:LaF3 single crystal around 1.05 μm and 1.32 μm

NASA Astrophysics Data System (ADS)

Xu, Bin; Huang, Xiaoxu; Lan, Jinglong; Lin, Zhi; Wang, Yi; Xu, Huiying; Cai, Zhiping; Moncorgé, Richard

2016-07-01

Calibrated room temperature polarized emission spectra recorded between 850 and 1400 nm and nearly free from any reabsorption effect are presented for the first time. A laser output power of 2.35 W is obtained at 1063.45 nm with a laser slope efficiency of about 56% by pumping an uncoated Nd:LaF3 single crystal with a fiber-coupled laser diode at 790 nm inside a standard two-mirror linear laser cavity. True dual-wavelength laser operation on two orthogonally polarized laser lines around 1040 and 1065 nm as well as continuous laser wavelength tuning around 1040 nm, 1048 nm and 1064 nm are also achieved for the first time by using either an intracavity etalon or a birefringent filter. Laser operation is finally obtained around 1330.73 nm with a maximum output power of 0.18 W and a laser slope efficiency of about 4% and simultaneous dual-wavelength laser operation at 1329.04 and 1359.67 nm is demonstrated by using a glass etalon.

Tunable, diode side-pumped Er: YAG laser

DOEpatents

Hamilton, Charles E.; Furu, Laurence H.

1997-01-01

A discrete-element Er:YAG laser, side pumped by a 220 Watt peak-power InGaAs diode array, generates >500 mWatts at 2.94 .mu.m, and is tunable over a 6 nm range near about 2.936 .mu.m. The oscillator is a plano-concave resonator consisting of a concave high reflector, a flat output coupler, a Er:YAG crystal and a YAG intracavity etalon, which serves as the tuning element. The cavity length is variable from 3 cm to 4 cm. The oscillator uses total internal reflection in the Er:YAG crystal to allow efficient coupling of the diode emission into the resonating modes of the oscillator. With the tuning element removed, the oscillator produces up to 1.3 Watts of average power at 2.94 .mu.m. The duty factor of the laser is 6.5% and the repetition rate is variable up to 1 kHz. This laser is useful for tuning to an atmospheric transmission window at 2.935 .mu.m (air wavelength). The laser is also useful as a spectroscopic tool because it can access several infrared water vapor transitions, as well as transitions in organic compounds. Other uses include medical applications (e.g., for tissue ablation and uses with fiber optic laser scalpels) and as part of industrial effluent monitoring systems.

Tunable, diode side-pumped Er:YAG laser

DOEpatents

Hamilton, C.E.; Furu, L.H.

1997-04-22

A discrete-element Er:YAG laser, side pumped by a 220 Watt peak-power InGaAs diode array, generates >500 mWatts at 2.94 {micro}m, and is tunable over a 6 nm range near about 2.936 {micro}m. The oscillator is a plano-concave resonator consisting of a concave high reflector, a flat output coupler, a Er:YAG crystal and a YAG intracavity etalon, which serves as the tuning element. The cavity length is variable from 3 cm to 4 cm. The oscillator uses total internal reflection in the Er:YAG crystal to allow efficient coupling of the diode emission into the resonating modes of the oscillator. With the tuning element removed, the oscillator produces up to 1.3 Watts of average power at 2.94 {micro}m. The duty factor of the laser is 6.5% and the repetition rate is variable up to 1 kHz. This laser is useful for tuning to an atmospheric transmission window at 2.935 {micro}m (air wavelength). The laser is also useful as a spectroscopic tool because it can access several infrared water vapor transitions, as well as transitions in organic compounds. Other uses include medical applications (e.g., for tissue ablation and uses with fiber optic laser scalpels) and as part of industrial effluent monitoring systems. 4 figs.

Extension of wavelength-modulation spectroscopy to large modulation depth for diode laser absorption measurements in high-pressure gases

NASA Astrophysics Data System (ADS)

Li, Hejie; Rieker, Gregory B.; Liu, Xiang; Jeffries, Jay B.; Hanson, Ronald K.

2006-02-01

Tunable diode laser absorption measurements at high pressures by use of wavelength-modulation spectroscopy (WMS) require large modulation depths for optimum detection of molecular absorption spectra blended by collisional broadening or dense spacing of the rovibrational transitions. Diode lasers have a large and nonlinear intensity modulation when the wavelength is modulated over a large range by injection-current tuning. In addition to this intensity modulation, other laser performance parameters are measured, including the phase shift between the frequency modulation and the intensity modulation. Following published theory, these parameters are incorporated into an improved model of the WMS signal. The influence of these nonideal laser effects is investigated by means of wavelength-scanned WMS measurements as a function of bath gas pressure on rovibrational transitions of water vapor near 1388 nm. Lock-in detection of the magnitude of the 2f signal is performed to remove the dependence on detection phase. We find good agreement between measurements and the improved model developed for the 2f component of the WMS signal. The effects of the nonideal performance parameters of commercial diode lasers are especially important away from the line center of discrete spectra, and these contributions become more pronounced for 2f signals with the large modulation depths needed for WMS at elevated pressures.

Ultracold atoms in an optical lattice one millimeter from air

NASA Astrophysics Data System (ADS)

Jervis, Dylan; Edge, Graham; Trotzky, Stefan; McKay, David; Thywissen, Joseph

2013-05-01

Over the past decade, ultracold atoms in optical lattices have shown to be versatile systems able to realize canonical Hamiltonians of condensed matter. High-resolution in-situ imaging of ultracold clouds has furthermore enabled thermometry, equation of state measurements, direct measurement of fluctuations, and unprecedented control. We report on microscopy of ultracold bosons and fermions in a novel configuration where the atoms are harmonically trapped 800 microns away from a 200 micron-thick vacuum window. This window also serves as a retro-reflecting mirror for an optical lattice, into which the atoms can be loaded. Two additional transverse standing waves complete the three-dimensional lattice setup. In free space, we have shown that laser cooling with 405 nm light, on the open 4S1/2-5P3/2 transition, allows for temperatures below the Doppler temperature of the 4S1/2-4P3/2 cycling transition at 767 nm. Microscopy with 405 nm light furthermore reduces the diffraction limit of in-situ imaging.

Spectroscopy of Vibrational States in Diatomic Iodine Molecules

NASA Astrophysics Data System (ADS)

Mulholland, Mary; Harrill, Charles H.; Smith, R. Seth

2015-04-01

This project is focused on understanding the vibrational structure of iodine, which is a homonuclear diatomic molecule. A 20 mW, 532 nm cw diode laser was used to selectively excite neutral iodine molecules to a higher energy electronic state. By performing spectroscopy on the transitions from this state to a lower energy electronic state, the data only showed those vibrational bands which connect the two electronic states. Since a number of vibrational levels are populated in the higher energy electronic state, the transitions to all of the allowed vibrational levels in the lower energy electronic state provided sufficient data to determine the vibrational structures of both states. Emission spectra were collected with an Ocean Optics USB4000 Compact CCD Spectrometer. The spectrometer had a range of 500 - 770 nm with a resolution of approximately 0.5 nm and was sensitive enough to resolve the vibrational states in diatomic iodine molecules. The results were compared to a simple harmonic oscillator model.

Laser spectroscopy of the 5P3/2 → 6Pj (j = 1/2 and 3/2) electric dipole forbidden transitions in atomic rubidium

NASA Astrophysics Data System (ADS)

Ponciano-Ojeda, F.; Hernández-Gómez, S.; Mojica-Casique, C.; Hoyos, L. M.; Flores-Mijangos, J.; Ramírez-Martínez, F.; Sahagún, D.; Jáuregui, R.; Jiménez-Mier, J.

2018-04-01

Doppler-free optical double-resonance spectroscopy is used to study the 5S1/2 → 5P3/2 → 6Pj (j = 3/2,1/2) excitation sequence in room-temperature rubidium atoms. This involves a 5S1/2 → 5P3/2 electric dipole preparation step followed by the 5P3/2 → 6Pj electric quadrupole excitation. The electric dipole forbidden transitions occur at 911.0 nm (j = 3/2) and 917.5 nm (j = 1/2). Production of atoms in the 6Pj states is detected by observing their direct decay to the ground state through emission of blue photons (λ ≈ 420 nm). A detailed experimental and theoretical study of the dependence on the relative linear polarizations of excitation beams is made. It is shown that specific electric quadrupole selection rules over magnetic quantum numbers are directly related to the relative orientation of the linear polarization of the excitation beams.

Recent development on high-power tandem-pumped fiber laser

NASA Astrophysics Data System (ADS)

Zhou, Pu; Xiao, Hu; Leng, Jinyong; Zhang, Hanwei; Xu, Jiangmin; Wu, Jian

2016-11-01

High power fiber laser is attracting more and more attention due to its advantage in excellent beam quality, high electricto- optical conversion efficiency and compact system configuration. Power scaling of fiber laser is challenged by the brightness of pump source, nonlinear effect, modal instability and so on. Pumping active fiber by using high-brightness fiber laser instead of common laser diode may be the solution for the brightness limitation. In this paper, we will present the recent development of various kinds of high power fiber laser based on tandem pumping scheme. According to the absorption property of Ytterbium-doped fiber, Thulium-doped fiber and Holmium-doped fiber, we have theoretically studied the fiber lasers that operate at 1018 nm, 1178 nm and 1150 nm, respectively in detail. Consequently, according to the numerical results we have optimized the fiber laser system design, and we have achieved (1) 500 watt level 1018nm Ytterbium-doped fiber laser (2) 100 watt level 1150 nm fiber laser and 100 watt level random fiber laser (3) 30 watt 1178 nm Ytterbium-doped fiber laser, 200 watt-level random fiber laser. All of the above-mentioned are the record power for the corresponded type of fiber laser to the best of our knowledge. By using the high-brightness fiber laser operate at 1018 nm, 1178 nm and 1150 nm that we have developed, we have achieved the following high power fiber laser (1) 3.5 kW 1090 nm Ytterbium-doped fiber amplifier (2) 100 watt level Thulium-doped fiber laser and (3) 50 watt level Holmium -doped fiber laser.

A Comparison Study of the Nonablative Fractional 1565-nm Er: glass and the Picosecond Fractional 1064/532-nm Nd: YAG Lasers in the Treatment of Striae Alba: A Split Body Double-Blinded Trial.

PubMed

Zaleski-Larsen, Lisa A; Jones, Isabela T; Guiha, Isabella; Wu, Douglas C; Goldman, Mitchel P

2018-05-09

Few effective treatments exist for striae alba, which are the mature stage of stretch marks. To evaluate the efficacy of the nonablative fractional 1,565-nm Er:glass and the picosecond fractional 1,064/532-nm Nd:YAG lasers in the treatment of striae alba. Twenty subjects with striae alba on the bilateral abdomen were treated with either the nonablative fractional 1565-nm Er:glass or the picosecond fractional 1,064/532-nm Nd:YAG laser, with a total of 3 treatments 3 weeks apart. A 31% (1.25/4) texture improvement was noted for both the fractional 1,565-nm Er:glass laser and the picosecond fractional 1,064/532-nm Nd:YAG laser. The degree of atrophy was improved by 30% (1.19/4) with the 1,565-nm Er:glass laser and 35% (1.38/4) with the picosecond 1,064/532-nm Nd:YAG laser. A 48% (1.9/4) subject overall assessment of improvement was noted with the fractional 1565-nm Er:glass laser and 45% (1.8/4) improvement with the picosecond fractional 1,064/532-nm Nd:YAG laser. There was no significant change in striae density with either laser. The picosecond laser was rated as less painful during all 3 sessions (p = .002) and had a shorter healing time (p = .035). The nonablative fractional 1,565-nm Er:glass and the picosecond fractional 1,064/532-nm Nd:YAG lasers were equally efficacious in improving striae alba.

Ultraviolet out-of-band radiation studies in laser tin plasma sources

NASA Astrophysics Data System (ADS)

Parchamy, Homaira; Szilagyi, John; Masnavi, Majid; Richardson, Martin

2017-11-01

Out-of-band long wavelength emission measurements from high power, high-repetition-rate extreme-ultra-violet lithography (EUVL) laser plasma sources are imperative to estimating heat deposition in EUV mirrors, and the impact of short wavelength light transported through the imaging system to the wafer surface. This paper reports a series of experiments conducted to measure the absolute spectral irradiances of laser-plasmas produced from planar tin targets over the wavelength region of 124 to 164 nm by 1.06 μm wavelength, 10 ns full-width-at-half-maximum Gaussian laser pulses. The use of spherical targets is relevant to the EUVL source scenario. Although plasmas produced from planar surfaces evolve differently, there is a close similarity to the evolution of current from 10.6 μm CO2 laser EUVL sources, which use a pre-pulse from a lower energy solid-state laser to melt and reform an initial spherical droplet into a thin planar disc target. The maximum of radiation conversion efficiency in the 124-164 nm wavelength band (1%/2πsr) occurs at the laser intensity of 1010 W cm-2. A developed collisional-radiative model reveals the strong experimental spectra that originate mainly from the 4d105p2-4d105s5p, 4d105p-4d105s resonance lines, and 4d95p-4d95s unresolved transition arrays from Sn III, Sn IV, and Sn V ions, respectively. The calculated conversion efficiencies using a 2D radiation-hydrodynamics model are in agreement with the measurements. The model predicts the out-of-band (100-400 nm) radiation conversion efficiencies generated by both 1.06 and 10.6 μm pulses. The 10.6 μm laser pulse produces a higher conversion efficiency (12%/2πsr) at the lower laser intensity of 109 W cm-2.

Direct nanopatterning of 100 nm metal oxide periodic structures by Deep-UV immersion lithography.

PubMed

Stehlin, Fabrice; Bourgin, Yannick; Spangenberg, Arnaud; Jourlin, Yves; Parriaux, Olivier; Reynaud, Stéphanie; Wieder, Fernand; Soppera, Olivier

2012-11-15

Deep-UV lithography using high-efficiency phase mask has been developed to print 100 nm period grating on sol-gel based thin layer. High efficiency phase mask has been designed to produce a high-contrast interferogram (periodic fringes) under water immersion conditions for 244 nm laser. The demonstration has been applied to a new developed immersion-compatible sol-gel layer. A sol-gel photoresist prepared from zirconium alkoxides caped with methacrylic acids was developed to achieve 50 nm resolution in a single step exposure. The nanostructures can be thermally annealed into ZrO(2). Such route considerably simplifies the process for elaborating nanopatterned surfaces of transition metal oxides, and opens new routes for integrating materials of interest for applications in the field of photocatalysis, photovoltaic, optics, photonics or microelectronics.

Nanometer-thick flat lens with adjustable focus

DOE Office of Scientific and Technical Information (OSTI.GOV)

Son, T. V.; Haché, A.; Ba, C. O. F.

2014-12-08

We report laser beam focusing by a flat, homogeneous film with a thickness of less than 100 nm. The effect relies on refractive index changes occurring in vanadium dioxide as it undergoes a phase transition from insulator to metal. Phase front curvature is achieved by means of temperature gradients, and adjustable focal lengths from infinity to 30 cm are attained.

Intense green emission from Tb3+- doped Teo2-Wo3-Geo2 glasses

NASA Astrophysics Data System (ADS)

Subrahmanyam, Tallam; Gopal, Kotalo Rama; Suvarna, Reniguntla Padma; Jamalaiah, Bungala Chinna

2018-04-01

Tb3+ -doped oxyfluoro tellurite (TWGTb) glasses were prepared by conventional melt quenching technique. The Judd-Ofelt theory has been applied to evaluate the Ωλ (λ=2,4,6) intensity parameters. The TWGTb glasses exhibit 5D3 → 7F5-3 and 5D4 → 7F6-0 transitions when excited at 316 nm wavelength. The variation of intensity of 5D4 → 7F5 (Green) and 5D3 → 7F4 (Blue) transitions and the green to blue (IG/IB) intensity ratios were studied as a function of Tb3+ ions concentration. The laser characteristic parameters such as effective bandwidth (Δλeff), stimulated emission cross-section (σe), gain bandwidth (σe×Δλeff) and optical gain (σe×τR) were determined using the emission spectra and radiative parameters. The luminescence decay profiles exhibit single-exponential nature for all the samples. Based on the experimental results we suggest that the 1.0 mol% of Tb3+-doped TWGTb glass could be the suitable laser host materials to emit intense green luminescence at 545 nm.

Multi-species laser absorption sensors for in situ monitoring of syngas composition

NASA Astrophysics Data System (ADS)

Sur, Ritobrata; Sun, Kai; Jeffries, Jay B.; Hanson, Ronald K.

2014-04-01

Tunable diode laser absorption spectroscopy sensors for detection of CO, CO2, CH4 and H2O at elevated pressures in mixtures of synthesis gas (syngas: products of coal and/or biomass gasification) were developed and tested. Wavelength modulation spectroscopy (WMS) with 1f-normalized 2f detection was employed. Fiber-coupled DFB diode lasers operating at 2325, 2017, 2290 and 1352 nm were used for simultaneously measuring CO, CO2, CH4 and H2O, respectively. Criteria for the selection of transitions were developed, and transitions were selected to optimize the signal and minimize interference from other species. For quantitative WMS measurements, the collision-broadening coefficients of the selected transitions were determined for collisions with possible syngas components, namely CO, CO2, CH4, H2O, N2 and H2. Sample measurements were performed for each species in gas cells at a temperature of 25 °C up to pressures of 20 atm. To validate the sensor performance, the composition of synthetic syngas was determined by the absorption sensor and compared with the known values. A method of estimating the lower heating value and Wobbe index of the syngas mixture from these measurements was also demonstrated.

Radiative data for highly excited 3d84d levels in Ni II from laboratory measurements and atomic calculations

NASA Astrophysics Data System (ADS)

Hartman, H.; Engström, L.; Lundberg, H.; Nilsson, H.; Quinet, P.; Fivet, V.; Palmeri, P.; Malcheva, G.; Blagoev, K.

2017-04-01

Aims: This work reports new experimental radiative lifetimes and calculated oscillator strengths for transitions from 3d84d levels of astrophysical interest in singly ionized nickel. Methods: Radiative lifetimes of seven high-lying levels of even parity in Ni II (98 400-100 600 cm-1) have been measured using the time-resolved laser-induced fluorescence method. Two-step photon excitation of ions produced by laser ablation has been utilized to populate the levels. Theoretical calculations of the radiative lifetimes of the measured levels and transition probabilities from these levels are reported. The calculations have been performed using a pseudo-relativistic Hartree-Fock method, taking into account core polarization effects. Results: A new set of transition probabilities and oscillator strengths has been deduced for 477 Ni II transitions of astrophysical interest in the spectral range 194-520 nm depopulating even parity 3d84d levels. The new calculated gf-values are, on the average, about 20% higher than a previous calculation and yield lifetimes within 5% of the experimental values.

Myocardium tissue ablation with high-peak-power nanosecond 1,064- and 532-nm pulsed lasers: influence of laser-induced plasma.

PubMed

Ogura, Makoto; Sato, Shunichi; Ishihara, Miya; Kawauchi, Satoko; Arai, Tunenori; Matsui, Takemi; Kurita, Akira; Kikuchi, Makoto; Ashida, Hiroshi; Obara, Minoru

2002-01-01

We investigated the mechanism and characteristics of porcine myocardium tissue ablation in vitro with nanosecond 1,064- and 532-nm pulsed lasers at laser intensities up to approximately 5.0 GW/cm(2). Particular attention was paid to study the influence of the laser-induced plasma on the ablation characteristics. The applicability of these two lasers to transmyocardial laser revascularization (TMLR) was discussed. Porcine myocardium tissue samples were irradiated with 1,064- and 532-nm, Q-switched Nd:YAG laser pulses, and the ablation depths were measured. The temporal profiles of the laser-induced optical emissions were measured with a biplanar phototube. For the ablated tissue samples, histological analysis was performed with an optical microscope and a polarization microscope. The ablation efficiency at 1,064 nm was higher than that at 532 nm. The ablation threshold at 1,064 nm (approximately 0.8 GW/cm(2)) was lower than that at 532 nm (approximately 1.6 GW/cm(2)), in spite of the lower absorption coefficient being expected at 1,064 nm. For the 1,064-nm laser-ablated tissues, thermal damage was very limited, while damage presumably caused by the mechanical effect was observed in most of the cases. For the 1,064-nm laser ablation, the ablation threshold was equal to the threshold of the laser-induced optical emission (approximately 0.8 GW/cm(2)), while for the 532-nm laser ablation, the optical emission threshold ( approximately 2.4 GW/cm(2)) was higher than the ablation threshold. We considered that for the 1,064-nm laser ablation, the tissue removal was achieved through a photodisruption process at laser intensities of > approximately 0.8 GW/cm(2). At laser intensities of > 3.0 GW/cm(2), however, the ablation efficiency decreased; this can be attributed to the absorption of incoming laser pulses by the plasma. For the 532-nm laser ablation, the tissue removal was achieved through a photothermal process at laser intensities of > approximately 1.6 GW/cm(2). At laser intensities of > 2.4 GW/cm(2), a photodisruption process may also contribute to the tissue removal, in addition to a photothermal process. With regard to the ablation rates, the 1,064-nm laser was more suitable for TMLR than the 532-nm laser. We concluded that the 1,064-nm Q-switched Nd:YAG laser would be a potential candidate for a laser source for TMLR because of possible fiber-based beam delivery, its compact structure, cost effectiveness, and easy maintenance. Animal trials, however, have to be carried out to evaluate the influence of the tissue damage. Copyright 2002 Wiley-Liss, Inc.

LIBS spectra of multi-component Al, Fe, Cu alloys and composite materials used for selected elements of armament and munition

NASA Astrophysics Data System (ADS)

Ostrowski, R.; Skrzeczanowski, W.; Rycyk, A.; CzyŻ, K.; Sarzyński, A.; Strzelec, M.; Jach, K.; Świerczyński, R.

2017-10-01

Spectral investigations in the UV-VIS range of selected Al, Cu, and Fe alloys and composite materials were performed using LIBS technique. The investigated objects were typical rifle cartridges, mortars, rocket launchers and samples of different type steel, Cu and Al alloys, as well as composite materials of special chemical composition. Two Nd:YAG lasers were applied: a short 4 ns, 60 mJ Brio Quantel/BigSky laser (1064 nm) and a long pulse 200/400 (up to 1000) µs ({ 2/4 up to 10 J) laser (1064 nm) constructed at the Institute of Optoelectronics MUT. This spectrochemical analysis was possible for Al, Cu, and Fe alloys objects for both lasers, and in case of composites only if the samples were irradiated by short laser pulse since in the experiment with the long pulse, all composite materials spectra, in general, were very similar to each other - they imitated a grey/black body spectra. For metal alloys in experiments with a short laser pulse only atomic spectra were observed while for long microsecond laser pulses molecular transitions have been registered for Al alloys. Electron temperatures of plasma created on different materials for short and long laser pulses were found on the base of Boltzmann plots. Temperatures are clearly higher for plasmas generated with a short laser pulse which results from much higher laser power density on the sample surface for short pulse and not from fluence which is 20-40 times larger for long pulse.

The Development and Deployment of a Ground-Based, Laser-Induced Fluorescence Instrument for the In Situ Detection of Iodine Monoxide Radicals

NASA Technical Reports Server (NTRS)

Thurlow, M. E.; Co, D. T.; O'Brien, A. S.; Hannun, R. A.; Lapson, L. B.; Hanisco, T. F.; Anderson, J. G.

2014-01-01

High abundances of iodine monoxide (IO) are known to exist and to participate in local photochemistry of the marine boundary layer. Of particular interest are the roles IO plays in the formation of new particles in coastal marine environments and in depletion episodes of ozone and mercury in the Arctic polar spring. This paper describes a ground-based instrument that measures IO at mixing ratios less than one part in 1012. The IO radical is measured by detecting laser-induced fluorescence at wavelengths longer that 500 nm. Tunable visible light is used to pump the A23/2 (v = 2) ? X23/2 (v = 0) transition of IO near 445 nm. The laser light is produced by a solid-state, Nd:YAG-pumped Ti:Sapphire laser at 5 kHz repetition rate. The laser-induced fluorescence instrument performs reliably with very high signal-to-noise ratios (>10) achieved in short integration times (<1 min). The observations from a validation deployment to the Shoals Marine Lab on Appledore Island, ME are presented and are broadly consistent with in situ observations from European Coastal Sites. Mixing ratios ranged from the instrumental detection limit (<1 pptv) to 10 pptv. These data represent the first in situ point measurements of IO in North America.

Diagnostics of Laser Produced Plume Under Carbon Nanotube Growth Conditions

NASA Technical Reports Server (NTRS)

Arepalli, Sivaram; Nikolaev, Pavel; Holmes, William; Scott, Carl D.

1999-01-01

This paper presents diagnostic data obtained from the plume of a graphite composite target during carbon nanotube production by the double-pulse laser oven method. The insitu emission spectrum (300 to 650 nm) is recorded at different locations upstream of the target and at different delay times from the lasers (IR and green). Spectral features are identified as emissions from C2 (Swan System: a (sup 3)pi(sub g) - delta (sup 3)pi(sub u) and C3 (Comet Head System: A (sup 1)pi(sub u) - chi (sup 1)sigma(sub u) (sup +). Experimental spectra are compared with computed spectra to estimate vibrational temperatures of excited state C2 in the range of 2500 to 4000 kappa The temporal evolution of the 510 nm band of C2 is monitored for two target positions in various locations which shows confinement of the plume in the inner tube and increase in plume velocity with temperature. The excitation spectra of C2 are obtained by using a dye laser to pump the (0,1) transition of the Swan System and collecting the Laser Induced Fluorescence signal from C2 These are used to obtain "ground-state" rotational and vibrational temperatures which are close to the oven temperature. Images of the plume are also collected and are compared with the spectral measurements.

Diode-pumped UV refractive surgery laser

NASA Astrophysics Data System (ADS)

Lin, Jui T.; Hwang, Ming-Yi; Huang, C. H.

1993-07-01

Ophthalmic applications of medical lasers have been extensively explored recently because of their market potential. Refractive surgical lasers represent one of the major development efforts due to the large population of eye disorders: about 160 million people in the USA and more than 2 billion worldwide. The first refractive laser developed was the ArF excimer laser at 193 nm in 1987 - 88 for a procedure called photorefractive keratectomy (PRK). More recently, solid state refractive lasers have also been explored for preliminary clinical trials. These lasers include Nd:YLF (picosecond at 1054 nm), doubled-Nd:YAG (nanosecond at 532 nm), Ho:YAG (microsecond at 2100 nm) and ultraviolet (UV) lasers generated from the harmonic of Ti:sapphire-laser (205 - 220 nm) and Nd:YAG (at 213 nm).

Pump-probe STM light emission spectroscopy for detection of photo-induced semiconductor-metal phase transition of VO2

NASA Astrophysics Data System (ADS)

Sakai, Joe; Katano, Satoshi; Kuwahara, Masashi; Uehara, Yoichi

2017-10-01

We attempted to observe pump-probe scanning tunneling microscopy (STM)-light emission (LE) from a VO2 thin film grown on a rutile TiO2(0 0 1) substrate, with an Ag tip fixed over a semiconducting domain. Laser pulses from a Ti:sapphire laser (wavelength 920 nm pulse width less than 1.5 ps) irradiated the tip-sample gap as pump and probe light sources. With a photon energy of 2.7 eV, suggesting phase transition from semiconducting monoclinic (M) to metallic rutile (R) phases in relation to the electronic band structure, faint LE was observed roughly 30 ps after the irradiation of the pump pulse, followed by retention for roughly 20 ps. The incident energy fluence of the pump pulse at the gap was five orders of magnitude lower than the threshold value for reported photo-induced M-R phase transition. The mechanism that makes it possible to reduce the threshold fluence is discussed.

Pump-probe STM light emission spectroscopy for detection of photo-induced semiconductor-metal phase transition of VO2.

PubMed

Sakai, Joe; Katano, Satoshi; Kuwahara, Masashi; Uehara, Yoichi

2017-10-11

We attempted to observe pump-probe scanning tunneling microscopy (STM)-light emission (LE) from a VO 2 thin film grown on a rutile TiO 2 (0 0 1) substrate, with an Ag tip fixed over a semiconducting domain. Laser pulses from a Ti:sapphire laser (wavelength 920 nm; pulse width less than 1.5 ps) irradiated the tip-sample gap as pump and probe light sources. With a photon energy of 2.7 eV, suggesting phase transition from semiconducting monoclinic (M) to metallic rutile (R) phases in relation to the electronic band structure, faint LE was observed roughly 30 ps after the irradiation of the pump pulse, followed by retention for roughly 20 ps. The incident energy fluence of the pump pulse at the gap was five orders of magnitude lower than the threshold value for reported photo-induced M-R phase transition. The mechanism that makes it possible to reduce the threshold fluence is discussed.

Strategy for improved NH2 detection in combustion environments using an Alexandrite laser

NASA Astrophysics Data System (ADS)

Brackmann, Christian; Zhou, Bo; Samuelsson, Per; Alekseev, Vladimir A.; Konnov, Alexander A.; Li, Zhongshan; Aldén, Marcus

2017-09-01

A new scheme for NH2 detection by means of laser-induced fluorescence (LIF) with excitation around wavelength 385 nm, accessible using the second harmonic of a solid-state Alexandrite laser, is presented. Detection of NH2 was confirmed by identification of corresponding lines in fluorescence excitation spectra measured in premixed NH3-air flames and on NH2 radicals generated through NH3 photolysis in a nonreactive flow at ambient conditions. Moreover, spectral simulations allow for tentative NH2 line identification. Dispersed fluorescence emission spectra measured in flames and photolysis experiments showed lines attributed to vibrational bands of the NH2 A2A1 ← X2B1 transition but also a continuous structure, which in flame was observed to be dependent on nitrogen added to the fuel, apparently also generated by NH2. A general conclusion was that fluorescence interferences need to be carefully considered for NH2 diagnostics in this spectral region. Excitation for laser irradiances up to 0.2 GW/cm2 did not result in NH2 fluorescence saturation and allowed for efficient utilization of the available laser power without indication of laser-induced photochemistry. Compared with a previously employed excitation/detection scheme for NH2 at around 630 nm, excitation at 385.7 nm showed a factor of 15 higher NH2 signal. The improved signal allowed for single-shot NH2 LIF imaging on centimeter scale in flame with signal-to-noise ratio of 3 for concentrations around 1000 ppm, suggesting a detection limit around 700 ppm. Thus, the presented approach for NH2 detection provides enhanced possibilities for characterization of fuel-nitrogen combustion chemistry.

Histologic evaluation of laser lipolysis: pulsed 1064-nm Nd:YAG laser versus cw 980-nm diode laser.

PubMed

Mordon, Serge; Eymard-Maurin, Anne Françoise; Wassmer, Benjamin; Ringot, Jean

2007-01-01

The use of the laser as an auxiliary tool has refined the traditional technique for lipoplasty. During laser lipolysis, the interaction between the laser and the fat produced direct cellular destruction before the suction, reduced bleeding, and promoted skin tightening. This study sought to perform a comparative histologic evaluation of laser lipolysis with the pulsed 1064-nm Nd:YAG laser versus a continuous 980-nm diode laser. A pulsed 1064-nm Nd:YAG (Smart-Lipo; Deka, Italy) and a CW 980-nm diode laser (Pharaon, Osyris, France) were evaluated at different energy settings for lipolysis on the thighs of a fresh cadaver. The lasers were coupled to a 600-microm optical fiber inserted in a 1-mm diameter cannula. Biopsy specimens were taken on irradiated and non-irradiated areas. Hematoxylin-erythrosin-safran staining and immunostaining (anti-PS100 polyclonal antibody) were performed to identify fat tissue damage. In the absence of laser exposures (control specimens), cavities created by cannulation were seen; adipocytes were round in appearance and not deflated. At low energy settings, tumescent adipocytes were observed. At higher energy settings, cytoplasmic retraction, disruption of membranes, and heat-coagulated collagen fibers were noted; coagulated blood cells were also present. For the highest energy settings, carbonization of fat tissue involving fibers and membranes was clearly seen. For equivalent energy settings, 1064-nm and 980-nm wavelengths gave similar histologic results. Laser lipolysis is a relatively new technique that is still under development. Our histologic findings suggest several positive benefits of the laser, including skin retraction and a reduction in intraoperative bleeding. The interaction of the laser with the tissue is similar at 980 nm and 1064 nm with the same energy settings. Because higher volumes of fat are removed with higher total energy, a high-power 980-nm diode laser could offer an interesting alternative to the 1064-nm Nd:YAG laser.

Investigations on nonlinear absorption and nonlinear refraction of a new photonic crystal using Z-scan

DOE Office of Scientific and Technical Information (OSTI.GOV)

Shetty, T. C. S., E-mail: tcsshetty@gmail.com; Department of Post Graduate Studies in Physics, St Aloysius College; Sandeep, K. M.

A new photonic material, (2E)-1-(3-chlorophenyl)-3-(2,4-dichlorophenyl)prop-2-en-1-one (DCPP) was synthesized and crystallised at room temperature. The functional groups of synthesised material were confirmed using FT-IR. The third order nonlinear optical (NLO) properties were investigated using Z-scan technique with 5 ns Nd:YAG laser pulses operating at a wavelength of 532 nm. Linear absorption spectrum of DCPP crystals shows an optical transmittance window and a lower cutoff wavelength of absorption at 380 nm. The direct transition band gap energy was determined using Tauc’s plot. The melting point and thermal stability of the crystal have been investigated by thermo gravimetric analysis/differential thermal analysis (TGA/DTA). Themore » Thermo gravimetric curve showed absence of any phase transition before melting point.« less

Endoluminal laser delivery mode and wavelength effects on varicose veins in an ex vivo model.

PubMed

Massaki, Ane B M N; Kiripolsky, Monika G; Detwiler, Susan P; Goldman, Mitchel P

2013-02-01

Endovenous laser ablation (EVLA) has been shown to be effective for the elimination of saphenous veins and associated reflux. Mechanism is known to be heat related, but precise way in which heat causes vein ablation is not completely known. This study aimed to determine the effects of various endovenous laser wavelengths and delivery modes on ex vivo human vein both macroscopically and microscopically. We also evaluated whether protected-tip fibers, consisting of prototype silica fibers with a metal tube over the distal end, reduced vein wall perforations compared with non-protected-tip fibers. An ex vivo EVLA model with human veins harvested during ambulatory phlebectomy procedures was used. Six laser fiber combinations were tested: 810 nm continuous wave (CW) diode laser with a flat tip fiber, 810 CW diode laser with a protected tip fiber, 1,320 nm pulsed Nd:YAG laser, 1,310 nm CW diode laser, 1,470 nm CW diode laser, and 2,100 nm pulsed Ho:YAG laser. Perforation or full thickness necrosis of a portion of the vein wall was observed in 5/11 (45%), 0/11 (0%), 3/22 (14%), 7/11 (64%), 4/6 (67%), and 5/10 (50%) of cross-sections of veins treated with the 810 nm CW diode laser with a flat tip fiber, the 810 CW diode laser with a protected tip fiber, the 1,320 nm pulsed Nd:YAG laser, the 1,310 nm CW diode laser, the 1,470 nm CW diode laser, and the 2,100 nm pulsed Ho:YAG laser, respectively. Our results have shown that the delivery mode, pulsed Nd:YAG versus CW, may be just as important as the wavelength. Therefore, the 1,310 nm CW laser may not be equivalent to the 1,320 nm pulsed laser. In addition, protected 810 nm fibers may be less likely to yield wall perforations than their non-protected counterparts. Copyright © 2012 Wiley Periodicals, Inc.

A study of the influence of Hg(6(3)P2) population in a low-pressure discharge on mercury ion emission at 194.2 nm

NASA Technical Reports Server (NTRS)

Maleki, L.; Blasenheim, B. J.; Janik, G. R.

1990-01-01

A low-pressure mercury-argon discharge, similar to the type existing in the mercury lamp for the trapped-ion standard, is probed with a new technique of laser spectroscopy to determine the influence of the Hg(6 3P(sub 2)) population on discharge emission. The discharge is excited with inductively coupled rf power. Variations in the intensity of emission lines in the discharge were examined as lambda = 546.1 nm light from a continuous wave (CW) laser excited the Hg(6 3P(sub 2)) to (7 3S (sub 1)) transition. The spectrum of the discharge viewed in the region of laser irradiation showed increased emission in lambda = 546.1, 435.8, 404.7, 253.7, and 194.2 nm lines. Other lines in Hg I exhibited a decrease in emission. When the discharge was viewed outside the region of laser irradiation, all lines exhibited an increased emission. Based on these results, it is concluded that the dominant mechanism for the excitation of higher lying levels of mercury is the the electron-impact excitation via the 3P(sub 2) level. The depopulation of this metastable is also responsible for the observed increase in the electron temperature when the laser irradiates the discharge. It is also concluded that the 3P(sub 2) metastable level of mercury does not play a significant role in the excitation of the 3P(sub 1/2) level of mercury ion.

Doppler-Free Spectroscopy of the {sup 1}S{sub 0}-{sup 3}P{sub 0} Optical Clock Transition in Laser-Cooled Fermionic Isotopes of Neutral Mercury

DOE Office of Scientific and Technical Information (OSTI.GOV)

Petersen, M.; Chicireanu, R.; Dawkins, S. T.

2008-10-31

We report direct laser spectroscopy of the {sup 1}S{sub 0}-{sup 3}P{sub 0} transition at 265.6 nm in fermionic isotopes of neutral mercury in a magneto-optical trap. Measurements of the frequency against the LNE-SYRTE primary reference using an optical frequency comb yield 1 128 575 290 808.4{+-}5.6 kHz in {sup 199}Hg and 1 128 569 561 139.6{+-}5.3 kHz in {sup 201}Hg. The uncertainty, allowed by the observation of the Doppler-free recoil doublet, is 4 orders of magnitude lower than previous indirect determinations. Mercury is a promising candidate for future optical lattice clocks due to its low sensitivity to blackbody radiation.

Ultraviolet 320 nm laser excitation for flow cytometry.

PubMed

Telford, William; Stickland, Lynn; Koschorreck, Marco

2017-04-01

Although multiple lasers and high-dimensional analysis capability are now standard on advanced flow cytometers, ultraviolet (UV) lasers (usually 325-365 nm) remain an uncommon excitation source for cytometry. This is primarily due to their cost, and the small number of applications that require this wavelength. The development of the Brilliant Ultraviolet (BUV fluorochromes, however, has increased the importance of this formerly niche excitation wavelength. Historically, UV excitation was usually provided by water-cooled argon- and krypton-ion lasers. Modern flow cytometers primary rely on diode pumped solid state lasers emitting at 355 nm. While useful for all UV-excited applications, DPSS UV lasers are still large by modern solid state laser standards, and remain very expensive. Smaller and cheaper near UV laser diodes (NUVLDs) emitting at 375 nm make adequate substitutes for 355 nm sources in many situations, but do not work as well with very short wavelength probes like the fluorescent calcium chelator indo-1. In this study, we evaluate a newly available UV 320 nm laser for flow cytometry. While shorter in wavelength that conventional UV lasers, 320 is close to the 325 nm helium-cadmium wavelength used in the past on early benchtop cytometers. A UV 320 nm laser was found to excite almost all Brilliant Ultraviolet dyes to nearly the same level as 355 nm sources. Both 320 nm and 355 nm sources worked equally well for Hoechst and DyeCycle Violet side population analysis of stem cells in mouse hematopoetic tissue. The shorter wavelength UV source also showed excellent excitation of indo-1, a probe that is not compatible with NUVLD 375 nm sources. In summary, a 320 nm laser module made a suitable substitute for conventional 355 nm sources. This laser technology is available in a smaller form factor than current 355 nm units, making it useful for small cytometers with space constraints. © 2017 International Society for Advancement of Cytometry. © 2017 International Society for Advancement of Cytometry.

Corneal tissue welding with infrared laser irradiation after clear corneal incision.

PubMed

Rasier, Rfat; Ozeren, Mediha; Artunay, Ozgür; Bahçecioğlu, Halil; Seçkin, Ismail; Kalaycoğlu, Hamit; Kurt, Adnan; Sennaroğlu, Alphan; Gülsoy, Murat

2010-09-01

The aim of this study was to investigate the potential of infrared lasers for corneal welding to seal corneal cuts done in an experimental animal model. Full-thickness corneal cuts on freshly enucleated bovine eyes were irradiated with infrared (809-nm diode, 980-nm diode, 1070-nm YLF, and 1980-nm Tm:YAP) lasers to get immediate laser welding. An 809-nm laser was used with the topical application of indocyanine green to enhance the photothermal interaction at the weld site. In total, 60 bovine eyes were used in this study; 40 eyes were used in the first part of the study for the determination of optimal welding parameters (15 eyes were excluded because of macroscopic carbonization, opacification, or corneal shrinkage; 2 eyes were used for control), and 20 eyes were used for further investigation of more promising lasers (YLF and Tm:YAP). Laser wavelength, irradiating power, exposure time, and spot size were the dose parameters, and optimal dose for immediate closure with minimal thermal damage was estimated through histological examination of welded samples. In the first part of the study, results showed that none of the applications was satisfactory. Full-thickness success rates were 28% (2 of 7) for 809-nm and for 980-nm diode lasers and 67% (2 of 3) for 1070-nm YLF and (4 of 6) for 1980-nm Tm:YAP lasers. In the second part of the study, YLF and Tm:YAP lasers were investigated with bigger sample size. Results were not conclusive but promising again. Five corneal incisions were full-thickness welded out of 10 corneas with 1070-nm laser, and 4 corneal incisions were partially welded out of 10 corneas with 1980-nm laser in the second part of the study. Results showed that noteworthy corneal welding could be obtained with 1070-nm YLF laser and 1980-nm Tm:YAP laser wavelengths. Furthermore, in vitro and in vivo studies will shed light on the potential usage of corneal laser welding technique.

Atomic Processes for XUV Lasers: Alkali Atoms and Ions

NASA Astrophysics Data System (ADS)

Dimiduk, David Paul

The development of extreme ultraviolet (XUV) lasers is dependent upon knowledge of processes in highly excited atoms. Described here are spectroscopy experiments which have identified and characterized certain autoionizing energy levels in core-excited alkali atoms and ions. Such levels, termed quasi-metastable, have desirable characteristics as upper levels for efficient, powerful XUV lasers. Quasi -metastable levels are among the most intense emission lines in the XUV spectra of core-excited alkalis. Laser experiments utilizing these levels have proved to be useful in characterizing other core-excited levels. Three experiments to study quasi-metastable levels are reported. The first experiment is vacuum ultraviolet (VUV) absorption spectroscopy on the Cs 109 nm transitions using high-resolution laser techniques. This experiment confirms the identification of transitions to a quasi-metastable level, estimates transition oscillator strengths, and estimates the hyperfine splitting of the quasi-metastable level. The second experiment, XUV emission spectroscopy of Ca II and Sr II in a microwave-heated plasma, identifies transitions from quasi-metastable levels in these ions, and provides confirming evidence of their radiative, rather than autoionizing, character. In the third experiment, core-excited Ca II ions are produced by inner-shell photoionization of Ca with soft x-rays from a laser-produced plasma. This preliminary experiment demonstrated a method of creating large numbers of these highly-excited ions for future spectroscopic experiments. Experimental and theoretical evidence suggests the CA II 3{ rm p}^5 3d4s ^4 {rm F}^circ_{3/2 } quasi-metastable level may be directly pumped via a dipole ionization process from the Ca I ground state. The direct process is permitted by J conservation, and occurs due to configuration mixing in the final state and possibly the initial state as well. The experiments identifying and characterizing quasi-metastable levels are compared to calculations using the Hartree-Fock code RCN/RCG. Calculated parameters include energy levels, wavefunctions, and transition rates. Based on an extension of this code, earlier unexplained experiments showing strong two-electron radiative transitions from quasi-metastable levels are now understood.

Direct writing of 150 nm gratings and squares on ZnO crystal in water by using 800 nm femtosecond laser.

PubMed

Liu, Jukun; Jia, Tianqing; Zhou, Kan; Feng, Donghai; Zhang, Shian; Zhang, Hongxin; Jia, Xin; Sun, Zhenrong; Qiu, Jianrong

2014-12-29

We present a controllable fabrication of nanogratings and nanosquares on the surface of ZnO crystal in water based on femtosecond laser-induced periodic surface structures (LIPSS). The formation of nanogrooves depends on both laser fluence and writing speed. A single groove with width less than 40 nm and double grooves with distance of 150 nm have been produced by manipulating 800 nm femtosecond laser fluence. Nanogratings with period of 150 nm, 300 nm and 1000 nm, and nanosquares with dimensions of 150 × 150 nm² were fabricated by using this direct femtosecond laser writing technique.

Q-Switched 660-nm Versus 532-nm Nd: YAG Laser for the Treatment for Facial Lentigines in Asian Patients: A Prospective, Randomized, Double-Blinded, Split-Face Comparison Pilot Study.

PubMed

Noh, Tai Kyung; Chung, Bo Young; Yeo, Un Cheol; Chang, SeoYoun; Lee, Mi Woo; Chang, Sung Eun

2015-12-01

Q-switched (QS) 532-nm lasers are widely used to treat solar lentigines. To compare the efficacy and safety of 660-nm and 532-nm QS neodymium-doped yttrium aluminum garnet (Nd:YAG) lasers in the treatment for lentigines in Asians. The halves of each face (randomly chosen) of 8 Korean Fitzpatrick Skin Type III-IV women with facial solar lentigines were treated with either 660-nm or 532-nm lasers. Pigmentation was measured objectively using a profilometric skin analysis tool and subjectively using the pigmentation area and severity index (PSI) score, global assessment of the aesthetic improvement scale (GAIS), and a patient satisfaction score at Weeks 4 and 8. Seven patients completed the study. No significant differences were found in the PSI, GAIS, patient satisfaction score, and melanin average score between the lasers. The melanin average level was significantly reduced by the 660-nm laser but not the 532-nm laser at Week 8 compared with the baseline. Both 660-nm and 532-nm QS Nd:YAG lasers effectively reduce pigmentation for up to 8 weeks with high patient satisfaction. The new 660-nm laser therefore increases the treatment options for lentigines in Asian skin.

Cavity-enhanced resonant photoacoustic spectroscopy with optical feedback cw diode lasers: A novel technique for ultratrace gas analysis and high-resolution spectroscopy.

PubMed

Hippler, Michael; Mohr, Christian; Keen, Katherine A; McNaghten, Edward D

2010-07-28

Cavity-enhanced resonant photoacoustic spectroscopy with optical feedback cw diode lasers (OF-CERPAS) is introduced as a novel technique for ultratrace gas analysis and high-resolution spectroscopy. In the scheme, a single-mode cw diode laser (3 mW, 635 nm) is coupled into a high-finesse linear cavity and stabilized to the cavity by optical feedback. Inside the cavity, a build-up of laser power to at least 2.5 W occurs. Absorbing gas phase species inside the cavity are detected with high sensitivity by the photoacoustic effect using a microphone embedded in the cavity. To increase sensitivity further, coupling into the cavity is modulated at a frequency corresponding to a longitudinal resonance of an organ pipe acoustic resonator (f=1.35 kHz and Q approximately 10). The technique has been characterized by measuring very weak water overtone transitions near 635 nm. Normalized noise-equivalent absorption coefficients are determined as alpha approximately 4.4x10(-9) cm(-1) s(1/2) (1 s integration time) and 2.6x10(-11) cm(-1) s(1/2) W (1 s integration time and 1 W laser power). These sensitivities compare favorably with existing state-of-the-art techniques. As an advantage, OF-CERPAS is a "zero-background" method which increases selectivity and sensitivity, and its sensitivity scales with laser power.

Electrodeless-discharge-vapor-lamp-based Faraday anomalous-dispersion optical filter.

PubMed

Sun, Qinqing; Zhuang, Wei; Liu, Zhiwen; Chen, Jingbiao

2011-12-01

We report an excited-state Faraday anomalous-dispersion optical filter operating on the rubidium 5P(3/2)-5D(5/2) transition (775.9 nm in vacuum) without the use of a pump laser. An electrodeless discharge vapor lamp is employed to replace the Rb vapor cell in a traditional Faraday anomalous-dispersion optical filter system. Atoms can be excited by power rather than a complex frequency-locked pump laser. A proof-of-concept experimental demonstration with a maximum transmission of 1.9% and a filter bandwidth of 650 MHz is presented. © 2011 Optical Society of America

Pump-probe differencing technique for cavity-enhanced, noise-canceling saturation laser spectroscopy.

PubMed

de Vine, Glenn; McClelland, David E; Gray, Malcolm B; Close, John D

2005-05-15

We present an experimental technique that permits mechanical-noise-free, cavity-enhanced frequency measurements of an atomic transition and its hyperfine structure. We employ the 532-nm frequency-doubled output from a Nd:YAG laser and an iodine vapor cell. The cell is placed in a folded ring cavity (FRC) with counterpropagating pump and probe beams. The FRC is locked with the Pound-Drever-Hall technique. Mechanical noise is rejected by differencing the pump and probe signals. In addition, this differenced error signal provides a sensitive measure of differential nonlinearity within the FRC.

Interaction of intense laser pulses with gas for two-color THz generation and remote magnetometry

NASA Astrophysics Data System (ADS)

Johnson, Luke A.

The interaction of intense laser pulses with atmospheric gases is studied in two contexts: (i) the generation of broadband terahertz radiation via two-color photoionization currents in nitrogen, and (ii) the generation of an electromagnetic wakefield by the induced magnetization currents of oxygen. (i) A laser pulse propagation simulation code was developed to investigate the radiation patterns from two-color THz generation in nitrogen. Understanding the mechanism for conical, two-color THz furthers the development of broadband THz sources. Two-color photoionization produces a cycle-averaged current driving broadband, conically emitted THz radiation. The THz emission angle is found to be determined by an optical Cherenkov effect, occurring when the front velocity of the ionization induced current source is greater than the THz phase velocity. (ii) A laser pulse propagating in the atmosphere is capable of exciting a magnetic dipole transition in molecular oxygen. The resulting transient current creates a co-propagating electromagnetic field behind the laser pulse, i.e. the wakefield, which has a rotated polarization that depends on the background magnetic field. This effect is analyzed to determine it's suitability for remote atmospheric magnetometry for the detection of underwater and underground objects. In the proposed approach, Kerr self-focusing is used to bring a polarized, high-intensity, laser pulse to focus at a remote detection site where the laser pulse induces a ringing in the oxygen magnetization. The detection signature for underwater and underground objects is the change in the wakefield polarization between different measurement locations. The magnetic dipole transition line that is considered is the b-X transition band of oxygen near 762 nm.

LED (660 nm) and laser (670 nm) use on skin flap viability: angiogenesis and mast cells on transition line.

PubMed

Nishioka, Michele A; Pinfildi, Carlos E; Sheliga, Tatiana Rodrigues; Arias, Victor E; Gomes, Heitor C; Ferreira, Lydia M

2012-09-01

Skin flap procedures are commonly used in plastic surgery. Failures can follow, leading to the necrosis of the flap. Therefore, many studies use LLLT to improve flap viability. Currently, the LED has been introduced as an alternative to LLLT. The objective of this study was to evaluate the effect of LLLT and LED on the viability of random skin flaps in rats. Forty-eight rats were divided into four groups, and a random skin flap (10 × 4 cm) was performed in all animals. Group 1 was the sham group; group 2 was submitted to LLLT 660 nm, 0.14 J; group 3 with LED 630 nm, 2.49 J, and group 4 with LLLT 660 nm, with 2.49 J. Irradiation was applied after surgery and repeated on the four subsequent days. On the 7th postoperative day, the percentage of flap necrosis was calculated and skin samples were collected from the viable area and from the transition line of the flap to evaluate blood vessels and mast cells. The percentage of necrosis was significantly lower in groups 3 and 4 compared to groups 1 and 2. Concerning blood vessels and mast cell numbers, only the animals in group 3 showed significant increase compared to group 1 in the skin sample of the transition line. LED and LLLT with the same total energies were effective in increasing viability of random skin flaps. LED was more effective in increasing the number of mast cells and blood vessels in the transition line of random skin flaps.

Spectroscopic studies of Nd3+ doped lead tungsten tellurite glasses for the NIR emission at 1062 nm

NASA Astrophysics Data System (ADS)

Venkateswarlu, M.; Mahamuda, Sk.; Swapna, K.; Prasad, M. V. V. K. S.; Srinivasa Rao, A.; Mohan Babu, A.; Shakya, Suman; Vijaya Prakash, G.

2015-01-01

Lead Tungsten Tellurite (LTT) glasses doped with different concentrations of Nd3+ ions were prepared by using the melt quenching technique to study the absorption, emission and decay spectral profiles with an aim to understand the lasing potentialities of these glasses. From the absorption spectra, the Judd-Ofelt (J-O) parameters are evaluated and in turn used to calculate the transition probability (AR), total transition probability (AT), radiative lifetime (τR) and branching ratios (βR) for prominent emission levels of Nd3+. The emission spectra recorded for LTT glasses gives three emission transitions 4F3/2 → 4I9/2, 4F3/2 → 4I11/2 and 4F3/2 → 4I13/2 for which effective band widths (ΔλP) and stimulated emission cross-sections (σse) are evaluated. Branching ratios (βR) measured for all the LTT glasses show that 4F3/2 → 4I11/2 transition is quite suitable for lasing applications. The intensity of emission spectra increases with increase in the concentrations of Nd3+ up to 1.0 mol% and beyond concentration quenching is observed. Relatively higher emission cross-sections and branching ratios observed for the present LTT glasses over the reported glasses suggests the feasibility of using LTT glasses for infrared laser applications. From the absorption, emission and decay spectral measurements, it was found that 1.0 mol% of Nd3+ ion concentration is aptly suitable for LTT glasses to give a strong NIR laser emission at 1062 nm.

Silver-gold alloy nanoparticles as tunable substrates for systematic control of ion-desorption efficiency and heat transfer in surface-assisted laser desorption/ionization.

PubMed

Lai, Samuel Kin-Man; Cheng, Yu-Hong; Tang, Ho-Wai; Ng, Kwan-Ming

2017-08-09

Systematically controlling heat transfer in the surface-assisted laser desorption/ionization (SALDI) process and thus enhancing the analytical performance of SALDI-MS remains a challenging task. In the current study, by tuning the metal contents of Ag-Au alloy nanoparticle substrates (AgNPs, Ag55Au45NPs, Ag15Au85NPs and AuNPs, ∅: ∼2.0 nm), it was found that both SALDI ion-desorption efficiency and heat transfer can be controlled in a wide range of laser fluence (21.3 mJ cm -2 to 125.9 mJ cm -2 ). It was discovered that ion detection sensitivity can be enhanced at any laser fluence by tuning up the Ag content of the alloy nanoparticle, whereas the extent of ion fragmentation can be reduced by tuning up the Au content. The enhancement effect of Ag content on ion desorption was found to be attributable to the increase in laser absorption efficiency (at 355 nm) with Ag content. Tuning the laser absorption efficiency by changing the metal composition was also effective in controlling the heat transfer from the NPs to the analytes. The laser-induced heating of Ag-rich alloy NPs could be balanced or even overridden by increasing the Au content of NPs, resulting in the reduction of the fragmentation of analytes. In the correlation of experimental measurement with molecular dynamics simulation, the effect of metal composition on the dynamics of the ion desorption process was also elucidated. Upon increasing the Ag content, it was also found that phase transition temperatures, such as melting, vaporization and phase explosion temperature, of NPs could be reduced. This further enhanced the desorption of analyte ions via phase-transition-driven desorption processes. The significant cooling effect on the analyte ions observed at high laser fluence was also determined to be originated from the phase explosion of the NPs. This study revealed that the development of alloy nanoparticles as SALDI substrates can constitute an effective means for the systematic control of ion-desorption efficiency and the extent of heat transfer, which could potentially enhance the analytical performance of SALDI-MS.

On pulse duration of self-terminating lasers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bokhan, P A

2011-02-28

The problem of the maximum pulse duration {tau}{sub max} of self-terminating lasers is considered. It is shown that the duration depends on the transition probability in the laser channel, on the decay rate of the resonant state in all other channels, and on the excitation rate of the metastable state. As a result, {tau}{sub max} is found to be significantly shorter than previously estimated. The criteria for converting the 'self-terminating' lasing to quasi-cw lasing are determined. It is shown that in the case of nonselective depopulation of the metastable state, for example in capillary lasers or in a fast flowmore » of the active medium gas, it is impossible to obtain continuous lasing. Some concrete examples are considered. It is established that in several studies of barium vapour lasers ({lambda} = 1.5 {mu}m) and nitrogen lasers ({lambda} = 337 nm), collisional lasing is obtained by increasing the relaxation rate of the metastable state in collisions with working particles (barium atoms and nitrogen molecules). (lasers)« less

Electronic properties of solids excited with intermediate laser power densities

NASA Astrophysics Data System (ADS)

Sirotti, Fausto; Tempo Beamline Team

Intermediate laser power density up to about 100 GW/cm2 is below the surface damage threshold is currently used to induce modification in the physical properties on short time scales. The absorption of a short laser pulse induces non-equilibrium electronic distributions followed by lattice-mediated equilibrium taking place only in the picosecond range. The role of the hot electrons is particularly important in several domains as for example fast magnetization and demagnetization processes, laser induced phase transitions, charge density waves. Angular resolved photoelectron spectroscopy measuring directly energy and momentum of electrons is the most adapted tool to study the electronic excitations at short time scales during and after fast laser excitations. The main technical problem is the space charge created by the pumping laser pulse. I will present angular resolved multiphoton photoemission results obtained with 800 nm laser pulses showing how space charge electrons emitted during fast demagnetization processes can be measured. Unable enter Affiliation: CNRS-SOLEIL Synchrotron L'Orme des Merisiers , Saint Aubin 91192 Gif sur Yvette France.

Widely tunable short-infrared thulium and holmium doped fluorozirconate waveguide chip lasers.

PubMed

Lancaster, D G; Gross, S; Withford, M J; Monro, T M

2014-10-20

We report widely tunable (≈ 260 nm) Tm(3+) and Ho(3+) doped fluorozirconate (ZBLAN) glass waveguide extended cavity lasers with close to diffraction limited beam quality (M(2) ≈ 1.3). The waveguides are based on ultrafast laser inscribed depressed claddings. A Ti:sapphire laser pumped Tm(3+)-doped chip laser continuously tunes from 1725 nm to 1975 nm, and a Tm(3+)-sensitized Tm(3+):Ho(3+) chip laser displays tuning across both ions evidenced by a red enhanced tuning range of 1810 to 2053 nm. We also demonstrate a compact 790 nm diode laser pumped Tm(3+)-doped chip laser which tunes from 1750 nm to 1998 nm at a 14% incident slope efficiency, and a beam quality of M(2) ≈ 1.2 for a large mode-area waveguide with 70 µm core diameter.

Power scaling of laser diode pumped Pr3+:LiYF4 cw lasers: efficient laser operation at 522.6 nm, 545.9 nm, 607.2 nm, and 639.5 nm.

PubMed

Gün, Teoman; Metz, Philip; Huber, Günter

2011-03-15

We report efficient cw laser operation of laser diode pumped Pr(3+)-doped LiYF4 crystals in the visible spectral region. Using two InGaN laser diodes emitting at λ(P)=443.9 nm with maximum output power of 1 W each and a 2.9-mm-long crystal with a doping concentration of 0.5%, output powers of 938 mW, 418 mW, 384 mW, and 773 mW were achieved for the laser wavelengths 639.5 nm, 607.2 nm, 545.9 nm, and 522.6 nm, respectively. The maximum absorbed pump powers were approximately 1.5 W, resulting in slope efficiencies of 63.6%, 32.0%, 52.1%, and 61.5%, as well as electro-optical efficiencies of 9.4%, 4.2%, 3.8%, and 7.7%, respectively. Within these experiments, laser diode-pumped laser action at 545.9 nm was demonstrated for what is believed to be the first time.

[Comparative investigation of underwater-LIBS using 532 and 1 064 nm lasers].

PubMed

Song, Jiao-Jian; Tian, Ye; Lu, Yuan; Li, Ying; Zheng, Rong-Er

2014-11-01

With the hope of applying laser induced breakdown spectroscopy (LIBS) to the ocean applications, the laser energy at 532 and 1 064 nm wavelength with 3 and 40 mj respectively was used, which was near their breakdown threshold. Extensive experimental investigations of LIBS from CaCl2 water solution were carried out in this paper using different laser wavelengths of 532 and 1 064 nm. The obtained results show that compared with the 532 nm laser, the 1 064 nm laser can induce the plasma in water with higher emission intensity and longer lifetime, while the reproducibility of LIBS signal under 1 064 nm laser is poorer. On the other hand, due to the different attenuation ratios of 532 and 1 064 nm laser energies in water, the LIBS signal of 1 064 nm laser decreases a lot within the transmission distance range 2-5 cm, while LIBS signal of 532 nm remains the same, because that the wavelength of 532 nm lies in the "transmission window" of the water solution. This study will provide valuable design considerations for the development of LIBS-sea system in near future.

Dy3+ doped tellurite glasses containing silver nanoparticles for lighting devices

NASA Astrophysics Data System (ADS)

Hua, Chenxiao; Shen, Lifan; Pun, Edwin Yue Bun; Li, Desheng; Lin, Hai

2018-04-01

Efficient warm yellowish-white fluorescence emissions of Dy3+ were observed in heavy metal germanium tellurite (HGT) glasses under the excitation of 454 nm. Further, the luminescence intensity of Dy3+ is increased by ∼29% accompanying the introduction of Ag NPs with diameter ∼7 nm when compared with that of the silver-free case, which is caused by the existence of localized surface plasmon resonance (LSPR). The larger net emission power, the more net emission photon number and the higher quantum yield in Dy2O3 doped HGT glasses containing Ag NPs (HGT-Ag) confirm the availability of utilizing laser. Presupposed fluorescence color trace reveals that white luminescence can be achieved when the intensity ratio between residual laser and Dy3+ emission reaches the appropriate range. The productive transition emissions and the tunable white fluorescence illustrate tellurite glasses embodying noble-metal NPs are a potential candidate for high-quality lighting devices.

On the O2(a1Δ) quenching by vibrationally excited ozone

NASA Astrophysics Data System (ADS)

Azyazov, V. N.; Mikheyev, P. A.; Heaven, M. C.

2010-09-01

The development of a discharge oxygen iodine laser (DOIL) requires efficient production of singlet delta oxygen (O2(a)) in electric discharge. It is important to understand the mechanisms by which O2(a) is quenched in these devices. To gain understanding of this mechanisms quenching of O2(a) in O(3P)/O2/O3/CO2/He/Ar mixtures has been investigated. Oxygen atoms and singlet oxygen molecules were produced by the 248 nm laser photolysis of ozone. The kinetics of O2(a) quenching were followed by observing the 1268 nm fluorescence of the O2 a --> X transition. Fast quenching of O2(a) in the presence of oxygen atoms and molecules was observed. The mechanism of the process has been examined using kinetic models, which indicate that quenching by vibrationally excited ozone is the dominant reaction.

Ho3+/Yb3+ co-doped TeO2-BaF2-Y2O3 glasses for ∼1.2 μm laser applications

NASA Astrophysics Data System (ADS)

Wang, Shunbin; Li, Chengzhi; Yao, Chuanfei; Jia, Shijie; Jia, Zhixu; Qin, Guanshi; Qin, Weiping

2017-02-01

Intense ∼1.2 μm fluorescence is observed in Ho3+/Yb3+ co-doped TeO2-BaF2-Y2O3 glasses under 915 nm laser diode excitation. The 1.2 μm emission can be ascribed to the transition 5I6→5I8 of Ho3+. With the introducing of BaF2, the content of OH in the glasses drops markedly, and the 1.2 μm emission intensity increases gradually as increasing the concentration percentage of BaF2. Furthermore, microstructured fibers based on the TeO2-BaF2-Y2O3 glasses are fabricated by using a rod-in-tube method, and a relative positive gain of ∼9.42 dB at 1175.3 nm is obtained in a 5 cm long fiber.

High-efficiency high-brightness diode lasers at 1470 nm/1550 nm for medical and defense applications

NASA Astrophysics Data System (ADS)

Gallup, Kendra; Ungar, Jeff; Vaissie, Laurent; Lammert, Rob; Hu, Wentao

2012-03-01

Diode lasers in the 1400 nm to 1600 nm regime are used in a variety of applications including pumping Er:YAG lasers, range finding, materials processing, aesthetic medical treatments and surgery. In addition to the compact size, efficiency, and low cost advantages of traditional diode lasers, high power semiconductor lasers in the eye-safe regime are becoming widely used in an effort to minimize the unintended impact of potentially hazardous scattered optical radiation from the laser source, the optical delivery system, or the target itself. In this article we describe the performance of high efficiency high brightness InP laser bars at 1470nm and 1550nm developed at QPC Lasers for applications ranging from surgery to rangefinding.

Comparison of 980-nm and 1070-nm in endovenous laser treatment (EVLT)

NASA Astrophysics Data System (ADS)

Topaloglu, Nermin; Tabakoglu, Ozgur; Ergenoglu, Mehmet U.; Gülsoy, Murat

2009-07-01

The use of endovenous laser treatment for varicose veins has been increasing in recent years. It is a safer technique than surgical vein stripping. Its complications (e.g. bruising, pain) are less than the complications of surgical vein stripping. But best parameters such as optimum wavelength, power, and application duration are still under investigation to clarify uncertainties about this technique. To prevent its complications and improve its clinical outcomes, the exact mechanism of it has to be known. The aim of this study is to investigate the effect of different laser wavelengths on endovenous laser therapy. In this study 980-nm diode laser and 1070-nm fiber laser were used. Human veins were irradiated with 980-nm and 1070-nm lasers at 8 W and 10 W to find the optimal power and wavelength. After laser application, remarkable shrinkage was observed. Inner and outer diameters of the veins also narrowed for both of the laser types. 10 W of 980-nm laser application led to better shrinkage results.

Separated oscillatory field microwave measurement of the n=2 3P1 to n=2 3P2 fine-structure interval of helium

NASA Astrophysics Data System (ADS)

Borbely, Joseph S.

2009-11-01

The fine-structure constant is a fundamental constant of nature that represents the strength of the coupling interaction between charged particles. Comparison of high-precision theory and high-precision experiment of the n=2 3PJ fine-structure intervals of helium will allow for a determination of the fine-structure constant. The 23P1(mJ=0)-to-23P 2(mJ=0) magnetic-dipole transition in helium is measured to be 2 291 177.53(35) kHz using Ramsey separated oscillatory fields. A thermal beam of 23S1 metastable helium atoms is produced in a DC discharge source and enters a chamber where a vertical DC magnetic field lifts the degeneracy of the mJ states. Initially, the 2 3S1(mJ=-1, 0, 1) states are equally populated. A linearly polarized 1083-nm diode laser drives the 23S 1(mJ=0) atoms up to the 23P0(m J=0) state, emptying the 23S1(mJ=0) state. A 15-ns laser pulse drives the 23S1(m J=+1)-to-23P1(mJ=0) transitions and this laser pulse is followed by two microwave pulses that drive the 2.29-GHz 23P1(mJ=0)-to-23P 2(mJ=0) transition. The atoms which undergo this microwave transition can spontaneously decay to the previously-emptied 23S 1(mJ=0) state. The 23P1(m J=0) state is forbidden to decay to the 23S1(m J=0) state since the transition has a zero electric-dipole matrix element. Therefore, any re-population of the 23S1(m J=0) state is a direct indication that the 2.29-GHz microwave transition has been driven. A linearly polarized 1083-nm diode laser detects the 2 3S1(mJ=0) atoms by exciting them up to the 2 3P0(mJ=0) state and the radiation from the resulting spontaneous decay is observed by focusing it onto a liquid-nitrogen-cooled InGaAs photodiode. The two microwave pulses are alternatively in phase or 180°out of phase and the difference of these signals versus microwave frequency leads to a Ramsey separated oscillatory field interference pattern.

Lidar Measurements of the Stratosphere and Mesosphere at the Biejing Observatory

NASA Astrophysics Data System (ADS)

Du, Lifang; Yang, Guotao; Cheng, Xuewu; Wang, Jihong

With the high precision and high spatial and temporal resolution, the lidar has become a powerful weapon of near space environment monitoring. This paper describes the development of the solid-state 532nm and 589nm laser radar, which were used to detect the wind field of Beijing stratosphere and mesopause field. The injection seeding technique and atomic absorption saturation bubble frequency stabilization method was used to obtain narrow linewidth of 532nm lidar, Wherein the laser pulse energy of 800mJ, repetition rate of 30Hz. The 589nm yellow laser achieved by extra-cavity sum-frequency mixing 1064nm and 1319nm pulse laser with KTP crystal. The base frequency of 1064nm and 1319nm laser adopted injection seeding technique and YAG laser amplification for high energy pulse laser. Ultimately, the laser pulse of 150mJ and the linewidth of 130MHz of 589nm laser was obtain. And after AOM crystal frequency shift, Doppler frequency discriminator free methods achieved of the measuring of high-altitude wind. Both of 532nm and 589nm lidar system for engineering design of solid-state lidar provides a basis, and also provide a solid foundation for the development of all-solid-state wind lidar.

Two-wavelength single laser CH and CH(4) imaging in a lifted turbulent diffusion flame.

PubMed

Namazian, M; Schmitt, R L; Long, M B

1988-09-01

A new technique has been developed which allows simultaneous 2-D mapping of CH and CH 4 in a turbulent methane flame. A flashlamp-pumped dye laser using two back mirrors produces output at 431.5 and 444 nm simultaneously. The 431.5-nm line is used to excite the (0, 0) band of the A(2)Delta-X(2)Pi system of CH, and the fluorescence of the (0, 1) transition is observed at 489 nm. Coincidentally, the spontaneous Raman scattering from CH(4) also occurs near 489 nm for a 431.5-nm excitation. To separate the CH(4) and CH contributions, the 444-nm line is used to produce a spontaneous Raman signal from CH(4) that is spectrally separated from the CH fluorescence. Subtraction of the signals generated by the 431.5- and 444-nm wavelength beams yields separate measurements of CH(4) and CH. Raman-scattered light records the instantaneous distribution of the fuel, and simultaneously the CH fluorescence indicates the location of the flame zone. The resulting composite images provide important insight on the interrelationship between fuel-air mixing and subsequent combustion.M. Namazian is with Altex Technologies Corporation, 109 Via De Tesoros, Los Gatos, California 95030; R. L. Schmitt is with Sandia National Laboratories, Combustion Research Facility, Livermore, California 94550; and M. B. Long is with Yale University, Department of Mechanical Engineering, New Haven, Connecticut 06520.

Laser-diode-pumped 1319-nm monolithic non-planar ring single-frequency laser

NASA Astrophysics Data System (ADS)

Wang, Qing; Gao, Chunqing; Zhao, Yan; Yang, Suhui; Wei, Guanghui; 2, Dongmei Hong

2003-10-01

Single-frequency 1319-nm laser was obtained by using a laser-diode-pumped monolithic Nd:YAG crystal with a non-planar ring oscillator (NPRO). When the NPRO laser was pumped by an 800-?m fiber coupled laser diode, the output power of the single-frequency 1319-nm laser was 220 mW, and the slope efficiency was 16%. With a 100-1m fiber coupled diode laser pumped, 99-mW single-frequency 1319-nm laser was obtained with a slope efficiency of 29%.

Analysis of frequency noise properties of 729nm extended cavity diode laser with unbalanced Mach-Zehnder interferometer

NASA Astrophysics Data System (ADS)

Pham, Tuan M.; Čížek, Martin; Hucl, Václav; Lazar, Josef; Hrabina, Jan; Řeřucha, Šimon; Lešundák, Adam; Obšil, Petr; Filip, Radim; Slodička, Lukáš; Číp, Ondřej

2016-12-01

We report on the frequency noise investigation of a linewidth-suppressed Extended Cavity Diode Laser (ECDL), working at 729 nm. Since the ECDL is intended as an excitation laser for the forbidden transition in a trapped and laser cooled 40Ca+ ion, an Hz-level linewidth is required. We present the experimental design that comprises a two-stage linewidth narrowing and a facility for frequency and noise analysis. The linewidth is first narrowed with a phase lock loop of the ECDL onto a selected component of an optical frequency comb where the frequency noise was suppressed with a fast electronic servo-loop controller that drives the laser injection current with a high bandwidth. The second stage comprises locking the laser onto a selected mode of a high-finesse passive optical cavity. The frequency analysis used an unbalanced Mach-Zehnder interferometer with a fiber spool inserted in the reference arm in order to give a general insight into the signal properties by mixing two separated beams, one of them delayed by the spool, and processing it with a spectral analyzer. Such a frequency noise analysis reveals what are the most significant noises contributions to the laser linewidth, which is a crucial information in field of ion trapping and cooling. The presented experimental results show the effect of the linewidth narrowing with the first stage, where the linewidth of ECDL was narrowed down to a kHz level.

Time integrated optical emission studies of the laser produced germanium plasma

NASA Astrophysics Data System (ADS)

Iqbal, Javed; Ahmed, R.; Baig, M. A.

2017-04-01

We present new time integrated data on the optical emission spectra of laser produced germanium plasma using a Q-switched Nd:YAG laser (1064 nm), power density up to about 5  ×  109 W cm-2 in conjunction with a set of five spectrometers covering a spectral range from 200 nm to 720 nm. Well resolved structure due to the 4p5s  →  4p2 transition array of neutral germanium and a few multiplets of singly ionized germanium have been observed. Plasma temperature has been determined in the range (9000-11 000) K using four different techniques; two line ratio method, Boltzmann plot, Saha-Boltzmann plot and Marotta’s technique whereas electron density has been deduced from the Stark broadened line profiles in the range (0.5-5.0)  ×  1017 cm-3, depending on the laser pulse energy to produce the germanium plasma. Full width at half maximum (FWHM) of a number of neutral and singly ionized germanium lines have been extracted by the Lorentzian fit to the experimentally observed line profiles. In addition, we have compared the experimentally measured relative line strengths for the 4p5s 3P0,1,2  →  4p2 3P0,1,2 multiplet with that calculated in the LS-coupling scheme revealing that the intermediate coupling scheme is more appropriate for the level designations in germanium.

Orange fiber laser for ophthalmology

NASA Astrophysics Data System (ADS)

Adachi, M.; Kojima, K.; Hayashi, K.

2007-02-01

For the light source of photocoagulators for ophthalmology, orange laser is more suitable than green laser because of low scattering loss by the crystalline lens, and low absorption by xanthophylls in the retina. We developed two orange fiber lasers (580 nm and 590 nm) to investigate the effect depending on the difference in the range of orange. The 580nm laser is composed of a 1160 nm fiber laser and a Periodically Polled Lithium Niobate (PPLN) crystal for second harmonic generation. The 1160 nm fiber laser beam is focused into the MgO-doped PPLN crystal whose length is 30 mm with 3-pass configuration. Continuous-wave 1.3 W output power of 580 nm was obtained with 5.8 W input power of 1160nm for the first time. The conversion efficiency was 22%. The band width of the second harmonic was 0.006 nm (FWHM). The 590 nm laser is almost the same as 580 nm laser source. In this case we used a Raman shift fiber to generate 1180 nm, and the output power of 590 nm was 1.4 W. We developed an evaluation model of photocoagulator system using these two laser sources. A 700 mW coagulation output power was obtained with this orange fiber laser photocoagulator system. This is enough power for the eye surgery. We have the prospect of the maintenance-free, long-life system that is completely air-cooled. We are planning to evaluate this photocoagulator system in order to investigate the difference between the two wavelengths at the field test.

Broadband white light emission from Ce:AlN ceramics: High thermal conductivity down-converters for LED and laser-driven solid state lighting

NASA Astrophysics Data System (ADS)

Wieg, A. T.; Penilla, E. H.; Hardin, C. L.; Kodera, Y.; Garay, J. E.

2016-12-01

We introduce high thermal conductivity aluminum nitride (AlN) as a transparent ceramic host for Ce3+, a well-known active ion dopant. We show that the Ce:AlN ceramics have overlapping photoluminescent (PL) emission peaks that cover almost the entire visible range resulting in a white appearance under 375 nm excitation without the need for color mixing. The PL is due to a combination of intrinsic AlN defect complexes and Ce3+ electronic transitions. Importantly, the peak intensities can be tuned by varying the Ce concentration and processing parameters, causing different shades of white light without the need for multiple phosphors or light sources. The Commission Internationale de l'Eclairage coordinates calculated from the measured spectra confirm white light emission. In addition, we demonstrate the viability of laser driven white light emission by coupling the Ce:AlN to a readily available frequency tripled Nd-YAG laser emitting at 355 nm. The high thermal conductivity of these ceramic down-converters holds significant promise for producing higher power white light sources than those available today.

Generation and use of high power 213 nm and 266 nm laser radiation and tunable 210-400 nm laser radiation with BBO crystal matrix array

DOEpatents

Gruen, Dieter M.

2000-01-01

A 213 nm laser beam is capable of single photon ablative photodecomposition for the removal of a polymer or biological material substrate. Breaking the molecular bonds and displacing the molecules away from the substrate in a very short time period results in most of the laser photon energy being carried away by the displaced molecules, thus minimizing thermal damage to the substrate. The incident laser beam may be unfocussed and is preferably produced by quintupling the 1064 nm radiation from a Nd:YAG solid state laser, i.e., at 213 nm. In one application, the 213 nm laser beam is expanded in cross section and directed through a plurality of small beta barium borate (BBO) crystals for increasing the energy per photon of the laser radiation directed onto the substrate. The BBO crystals are arranged in a crystal matrix array to provide a large laser beam transmission area capable of accommodating high energy laser radiation without damaging the BBO crystals. The BBO crystal matrix array may also be used with 266 nm laser radiation for carrying out single or multi photon ablative photodecomposition. The BBO crystal matrix array may also be used in an optical parametric oscillator mode to generate high power tunable laser radiation in the range of 210-400 nm.

Supersonic Mass Flux Measurements via Tunable Diode Laser Absorption and Non-Uniform Flow Modeling

NASA Technical Reports Server (NTRS)

Chang, Leyen S.; Strand, Christopher L.; Jeffries, Jay B.; Hanson, Ronald K.; Diskin, Glenn S.; Gaffney, Richard L.; Capriotti, Diego P.

2011-01-01

Measurements of mass flux are obtained in a vitiated supersonic ground test facility using a sensor based on line-of-sight (LOS) diode laser absorption of water vapor. Mass flux is determined from the product of measured velocity and density. The relative Doppler shift of an absorption transition for beams directed upstream and downstream in the flow is used to measure velocity. Temperature is determined from the ratio of absorption signals of two transitions (lambda(sub 1)=1349 nm and lambda(sub 2)=1341.5 nm) and is coupled with a facility pressure measurement to obtain density. The sensor exploits wavelength-modulation spectroscopy with second-harmonic detection (WMS-2f) for large signal-to-noise ratios and normalization with the 1f signal for rejection of non-absorption related transmission fluctuations. The sensor line-of-sight is translated both vertically and horizontally across the test section for spatially-resolved measurements. Time-resolved measurements of mass flux are used to assess the stability of flow conditions produced by the facility. Measurements of mass flux are within 1.5% of the value obtained using a facility predictive code. The distortion of the WMS lineshape caused by boundary layers along the laser line-of-sight is examined and the subsequent effect on the measured velocity is discussed. A method for correcting measured velocities for flow non-uniformities is introduced and application of this correction brings measured velocities within 4 m/s of the predicted value in a 1630 m/s flow.

Comparison of the effects of 665 nm low level diode Laser Hat versus and a combination of 665 nm and 808nm low level diode Laser Scanner of hair growth in androgenic alopecia.

PubMed

Barikbin, Behrooz; Khodamrdi, Zeinab; Kholoosi, Leila; Akhgri, Mohammad Reza; Haj Abbasi, Majid; Hajabbasi, Mojgan; Razzaghi, Zahra; Akbarpour, Samaneh

2017-05-17

This study aimed to evaluate the effectiveness of a combined set of low level diode laser scanner (665 nm and 808nm) on hair growth, and assessment of safety and effectiveness of a new laser scanner on hair growth treatment procedure in androgenic alopecia. 90 patients (18 to 70 years) with androgenic alopecia were randomized into three groups. The first group (n=30) received 655 nm red light using laser hat, the second group (n=30) received 655 nm red laser plus 808 nm infrared laser using a laser scanner of hair growth device (with the patent number: 77733) and the third group (n=30) received no laser as the control group. Patients in laser scanner group had better results and showed a higher increase in terminal hair density compared with laser hat group (mean of 9.61 versus 9.16 per cm 2 ). We found significant decrease in terminal hair density from baseline in control group (mean -1.8 per cm 2 , p<0.0001). Results showed a statistically significant improvement in the laser scanner of the hair growth group compared with laser hat and the control group. The study showed that treatment with new laser devise had a promising result without any observable adverse effects.

Femtosecond Optical and X-Ray Measurement of the Semiconductor-to-Metal Transition in VO2

NASA Astrophysics Data System (ADS)

Cavalleri, Andrea; Toth, Csaba; Squier, Jeff; Siders, Craig; Raksi, Ferenc; Forget, Patrick; Kieffer, Jean-Claude

2001-03-01

While the use of ultrashort visible pulses allows access to ultrafast changes in the optical properties during phase transitions, measurement of the correlation between atomic movement and electronic rearrangement has proven more elusive. Here, we report on the conjunct measurement of ultrafast electronic and structural dynamics during a semiconductor-to-metal phase transition in VO2. Rearrangement of the unit cell from monoclinic to rutile (measured by ultrafast x-ray diffraction) is accompanied by a sharp increase in the electrical conductivity and perturbation of the optical properties (measured with ultrafast visible spectroscopy). Ultrafast x-ray diffraction experiments were performed using femtosecond bursts of Cu-Ka from a laser generated plasma source. A clear rise of the diffraction signal originating from the impulsively generated metallic phase was observable on the sub-picosecond timescale. Optical experiments were performed using time-resolved microscopy, providing temporally and spatially resolved measurements of the optical reflectivity at 800 nm. The data indicate that the reflectivity of the low-temperature semiconducting solid is driven to that of the equilibrium, high-temperature metallic phase within 400 fs after irradiation with a 50-fs laser pulse at fluences in excess of 10 mJ/cm2. In conclusion, the data presented in this contribution suggest that the semiconductor-to-metal transition in VO2 occurs within 500 fs after laser-irradiation. A nonthermal physical mechanism governs the re-arrangement.

A highly integrated single-mode 1064 nm laser with 8.5 kHz linewidth for dual-wavelength active optical clock

NASA Astrophysics Data System (ADS)

Shi, Tiantian; Pan, Duo; Chang, Pengyuan; Shang, Haosen; Chen, Jingbiao

2018-04-01

Without exploiting any frequency selective elements, we have realized a highly integrated, single-mode, narrow-linewidth Nd:YAG 1064 nm laser, which is end-pumped by the 808.6 nm diode laser in an integrated invar cavity. It turns out that each 1064 nm laser achieves a most probable linewidth of 8.5 kHz by beating between two identical laser systems. The output power of the 1064 nm laser increases steadily as the 808.6 nm pump power is raised, which can be up to 350 mW. Moreover, the resonant wavelength of cavity grows continuously in a certain crystal temperature range. Such a 1064 nm laser will be frequency stabilized to an ultrastable cavity by using the Pound-Drever-Hall technique and used as the good cavity laser to lock the main cavity length of 1064/1470 nm good-bad cavity dual-wavelength active optical clock.

Amplification of spontaneous emission on sodium D-lines using nonresonance broadband optical pumping

NASA Astrophysics Data System (ADS)

Petukhov, T. D.; Evtushenko, G. S.; Tel'minov, E. N.

2018-04-01

This work describes an experimental study of obtaining the amplified spontaneous emission (ASE) on sodium D-lines using nonresonance broadband optical pumping. ASE is observed at transitions D2 and D1 line: 589 nm (32 P3/2 - 32 S1/2) and 589.6 nm (32 P1/2 - 32 S1/2). The active medium was pumped by the dye laser with FWHM of 5 nm, maximum radiation in the range 584.5-586.5 nm, and pulse energy above 2 mJ. The working temperature of the active medium was 260 °C, initial pressure of buffer gas-helium was 300 torr (operating pressure - 500 torr). A change in the absorption spectra at D lines at different temperatures of the active medium and buffer gas pressures was observed

Time-synchronized continuous wave laser-induced fluorescence on an oscillatory xenon discharge.

PubMed

MacDonald, N A; Cappelli, M A; Hargus, W A

2012-11-01

A novel approach to time-synchronizing laser-induced fluorescence measurements to an oscillating current in a 60 Hz xenon discharge lamp using a continuous wave laser is presented. A sample-hold circuit is implemented to separate out signals at different phases along a current cycle, and is followed by a lock-in amplifier to pull out the resulting time-synchronized fluorescence trace from the large background signal. The time evolution of lower state population is derived from the changes in intensity of the fluorescence excitation line shape resulting from laser-induced fluorescence measurements of the 6s(')[1/2](1)(0)-6p(')[3/2](2) xenon atomic transition at λ = 834.68 nm. Results show that the lower state population oscillates at twice the frequency of the discharge current, 120 Hz.

Toward compact and ultra-intense laser-based soft x-ray lasers

NASA Astrophysics Data System (ADS)

Sebban, S.; Depresseux, A.; Oliva, E.; Gautier, J.; Tissandier, F.; Nejdl, J.; Kozlova, M.; Maynard, G.; Goddet, J. P.; Tafzi, A.; Lifschitz, A.; Kim, H. T.; Jacquemot, S.; Rousseau, P.; Zeitoun, P.; Rousse, A.

2018-01-01

We report here recent work on an optical field ionized (OFI), high-order harmonic-seeded EUV laser. The amplifying medium is a plasma of nickel-like krypton obtained by OFI when focusing a 1 J, 30 fs, circularly-polarized, infrared pulse into a krypton-filled gas cell or krypton gas jet. The lasing transition is the 3d94d (J = 0) → 3d94p (J = 1) transition of Ni-like krypton ions at 32.8 nm and is pumped by collisions with hot electrons. The gain dynamics was probed by seeding the amplifier with a high-order harmonic pulse at different delays. The gain duration monotonically decreased from 7 ps to an unprecedented shortness of 450 fs full width at half-maximum as the amplification peak rose from 150 to 1200 with an increase of the plasma density from 3 × 1018 to 1.2 × 1020 cm-3. The integrated energy of the EUV laser pulse was also measured, and found to be around 2 μJ. It is to be noted that in the ASE mode, longer amplifiers were achieved (up to 2 cm), yielding EUV outputs up to 14 μJ.

Vibrational wave packets in the B 1Πu and D 1Σu+ states of Cs2: Determination of improved Cs2+(X) and Cs2(B) spectroscopic constants

NASA Astrophysics Data System (ADS)

Oldenburg, A. L.; John, P. C.; Eden, J. G.

2000-12-01

Vibrational wave packets in the B 1Πu and D 1Σu+ excited states of Cs2 have been studied on the ˜100 fs time scale by pump-probe laser spectroscopy. The temporal behavior of the wave packets was monitored by photoionizing the electronically excited molecule with a time-delayed probe pulse and recording the time and energy-integrated photoelectron signal as a function of time delay between the pump and probe pulses. For the B 1Σu+ experiments, wave packets were produced by exciting the B 1Σu+←X 1Σg+ transition in the ˜740-790 nm region and subsequently detected by photoionizing the molecule at wavelengths between 565 nm and 600 nm. By simulating the experimentally observed transients with the density matrix formalism (and explicitly accounting for laser chirp and |Δv|>1 coherences), improved values for the equilibrium internuclear separation for the Cs2(B1Πu) state and Te for the Cs2+(X) state were determined to be Re(B 1Πu)=4.93±0.03 Å and Te[Cs2+(X)]=29 930±100 cm-1, respectively. Similar experiments were conducted for the D 1Σu+ state. Wave packets composed of vibrational levels (v'≈40-50) perturbed by the bound 2 3Πou state were produced on the D 1Σu+ potential surface by driving the D 1Σu+←X 1Σg+ transition in the 575-610 nm spectral interval.

Blood absorption during 970 and 1470 nm laser radiation in vitro.

PubMed

Shaydakov, E; Ilyukhin, E; Rosukhovskiy, D

2015-10-01

Soon after introduction of water lasers in medical practice for EVLA, less power and energy line density have been used. However, there are no experimental grounds for different energy modes and there is no clear evidence for a difference in the effect of the two wavelengths dealt with in this study. The goal of this study was to evaluate the temperature profile of various laser action modes with testing devices. Three experimental testing devices consisted of cylinders filled with whole donor blood and a set of temperature sensors installed in different positions. We have determined the range of temperatures around the fiber tip of 970 and 1470 nm lasers. The average temperature of 970 nm laser at 1 mm distance along the axis from the fiber tip substantially differed from that of 1470 nm laser, power being equal. Statistically substantial differences were found in endovenous laser ablation simulation in vitro for the 970 nm and 1470 nm laser radiation. Similar temperatures can be reached with 970 nm lasers if power is increased.

New alternatives for laser vaporization of the prostate: experimental evaluation of a 980-, 1,318- and 1,470-nm diode laser device.

PubMed

Wezel, Felix; Wendt-Nordahl, Gunnar; Huck, Nina; Bach, Thorsten; Weiss, Christel; Michel, Maurice Stephan; Häcker, Axel

2010-04-01

Several diode laser systems were introduced in recent years for the minimal-invasive surgical therapy of benign prostate enlargement. We investigated the ablation capacities, hemostatic properties and extend of tissue necrosis of different diode lasers at wavelengths of 980, 1,318 and 1,470 nm and compared the results to the 120 W GreenLight HPS laser. The laser devices were evaluated in an ex vivo model using isolated porcine kidneys. The weight difference of the porcine kidneys after 10 min of laser vaporization defined the amount of ablated tissue. Blood loss was measured in blood-perfused kidneys following laser vaporization. Histological examination was performed to assess the tissue effects. The side-firing 980 and 1,470 nm diode lasers displayed similar ablative capacities compared to the GreenLight HPS laser (n.s.). The 1,318-nm laser, equipped with a bare-ended fiber, reached a higher ablation rate compared to the other laser devices (each P < 0.05). A calculated 'output power efficiency per watt' revealed that the 1,318-nm laser with a bare-ended fiber reached the highest rate compared to the side-firing devices (each P < 0.0001). All three diode lasers showed superior hemostatic properties compared to the GreenLight HPS laser (each P < 0.01). The extend of morphological tissue necrosis was 4.62 mm (1,318 nm), 1.30 mm (1,470 nm), 4.18 mm (980 nm) and 0.84 mm (GreenLight HPS laser), respectively. The diode lasers offered similar ablative capacities and improved hemostatic properties compared to the 120 W GreenLight HPS laser in this experimental ex vivo setting. The higher tissue penetration of the diode lasers compared to the GreenLight HPS laser may explain improved hemostasis.

Silicon Carbide Defect Qubits/Quantum Memory with Field-Tuning: OSD Quantum Science and Engineering Program (QSEP)

DTIC Science & Technology

2017-08-01

accessories for mounting e. Laser power supply f. TEC power supply 12. Optical filters from SEMROCK ®, THORLABS Inc., EDMUND OPTICS® a. 532-nm, laser...line filter ( SEMROCK ®) b. 550-nm, hard-coated, short-pass filter (THORLABS Inc.) c. 532-nm long-pass filter ( SEMROCK ®) d. 808-nm laser-line filter... SEMROCK ®) e. 850-nm /10-nm full width at half maximum (FWHM) bandpass filter ( SEMROCK ®) f. 980-nm bandpass filter ( SEMROCK ®) g. 976-nm laser-line

Vibrational Spectroscopy of Laser Cooled CaH

DTIC Science & Technology

2015-10-28

about 1 mW 369 nm laser with a bandpass filter ( Semrock 395/20 nm) that reflects the 21 399 nm laser and transmits the 369 nm laser, which are sent along...and the back mirror is a flat broadband 67 ( Semrock MaxMirror) mirror that has over 99% reflectivity over a wide range as shown in Fig. 28. The lasers

A 15 W 1152 nm Raman fiber laser with 6 nm spectral width for Ho3+-doped crystal's pumping source

NASA Astrophysics Data System (ADS)

Chen, Xiuyan; Jiang, Huawei

2016-12-01

A 11.5 W 1152 nm Raman fiber laser with 6 nm spectral width was demonstrated based on the resonator constructed with one fiber loop mirror and one fiber Bragg grating. By mans of experimental measurement and theoretical calculation, the reflectivity of the fiber loop mirror was confirmed as 0.93. The Yb3+-doped 1090 nm fiber length was about 5 m. When the maximum pumping power of 976 nm laser was 54.8 W, 32.2 W 1090 nm laser was obtained and the optical to optical conversion efficiency from 1090 nm to 1152 nm light was 48%. Finally, the 1152 nm Raman fiber laser was used for pumping Ho3+:LLF crystal, and the 1194 nm fluorescence emission peak was detected for the first time.

40nm tunable multi-wavelength fiber laser

NASA Astrophysics Data System (ADS)

Jia, Qingsong; Wang, Tianshu; Zhang, Peng; Dong, Keyan; Jiang, Huilin

2014-12-01

A Brillouin-Erbium multi-wavelength tunable fiber laser at C-band is demostrated. A 10 km long singlemode fiber(SMF), a 6 m long Erbium-doped fiber, two couplers, a wavelength division multiplexer, a isolator, an optical circulator, a 980nm pump laser and a narrow linewidth tunable laser are included in the structure. A segment of 10 km-long single-mode fiber (SMF) between the two ports of a 1×2 coupler is used as Brillouin gain. Ebiumdoped fiber amplifier (EDFA) consists of a segment of 6m er-doped fiber pumped by 980nm laser dioder . A narrow linewidth tunable laser from 1527 to 1607 nm as Brillouin bump, At the Brillouin pump power of 8mW and the 980 nm pump power of 400 mw, 16 output channels with 0.08 nm spacing and tuning range of 40 nm from 1527 nm to 1567 nm are achieved. We realize the tunable output of wavelength by adjusting the 980 nm pump power and the Brillouin pump wavelength. Stability of the multiwavelength fiber laser is also observed.

New, efficient, room temperature mid-infrared laser at 3.9 mu m in holmium:barium yttrium fluoride and visible praseodymium:lithium yttrium fluoride laser for holography

NASA Astrophysics Data System (ADS)

Tabirian, Anna Murazian

This dissertation describes a series of experiments and theoretical studies, which led to the development of two new solid state laser systems: efficient, room temperature mid-infrared solid state laser at 3.9 μm in Ho 3+ doped BaY2F8 and visible Pr:LiYF4 laser at 640 mn for holography. The 3.9 μm laser wavelength matches the peak of mid-IR atmospheric transmission window, which makes it very important for multiple applications such as remote sensing, imaging, IR countermeasures, eye-safe lidars and environmental agent detection. We present the results of spectroscopic evaluations and numerical modeling of energy transfer processes between rare earth ions of Ho3+ doped in two host laser materials: BaY2F8 and LiYF 4. The 3.9 μm laser is based on transition with upper laser lifetime considerably shorter than lower level lifetime, which in general leads to self-terminating laser action in the cw mode or at high repetition rates. Therefore, three different pumping and lasing schemes, that could allow overcoming these limitations have been suggested and studied. First, cascade laser action at 1.4 μm and 3.9 μm was achieved with low thresholds and near-theoretical quantum efficiency in Ho3+ doped BaY2F8 pumped at 532 nm by a Q- switched frequency doubled Nd:YAG laser. Next, the feasibility of achieving 3.9 μm laser with cw resonant cascade pumping at 750 mn by a Ti:Sapphire laser was studied. New energy transfer process, such as upconversion from terminal level of the 3.9 μm laser was observed in high concentration Ho3+ doped BaY2F 8. Finally, we proposed to use high-energy flashlamp pumped tunable Cr:LiSAF laser operating in long pulse regime for the direct pumping of the upper level of the 3.9 μm laser. Pulsed laser oscillation at 3.9 μm is demonstrated in Ho3+ doped BaY2F8 with low threshold of 3 mJ and a slope efficiency of 14.5% with maximal energy of 30 mJ. The second part of the thesis describes the design and the development of the visible Pr:LiYF4 laser for holography at 640 nm resonantly pumped by the frequency-doubled flashlamp pumped tunable Cr:LiSAF laser at 444 nm.

Laser Application in Dentistry: Irradiation Effects of Nd:YAG 1064 nm and Diode 810 nm and 980 nm in Infected Root Canals-A Literature Overview.

PubMed

Saydjari, Yves; Kuypers, Thorsten; Gutknecht, Norbert

2016-01-01

Objective. In endodontics, Nd:YAG laser (1064 nm) and diode laser (810 nm and 980 nm) devices are used to remove bacteria in infected teeth. A literature review was elaborated to compare and evaluate the advantages and disadvantages of using these lasers. Methods. Using combined search terms, eligible articles were retrieved from PubMed and printed journals. The initial search yielded 40 titles and 27 articles were assigned to full-text analysis. The studies were classified based upon laser source, laser energy level, duration/similarity of application, and initial and final bacterial count at a minimum of 20 prepared root canals. Part of the analysis was only reduced microorganisms and mechanically treated root canals upon preparation size of ISO 30. All studies were compared to evaluate the most favorable laser device for best results in endodontic therapy. Results. A total of 22 eligible studies were found regarding Nd:YAG laser 1064 nm. Four studies fulfilled all demanded criteria. Seven studies referring to the diode laser 980 nm were examined, although only one fulfilled all criteria. Eleven studies were found regarding the diode laser 810 nm, although only one study fulfilled all necessary criteria. Conclusions. Laser therapy is effective in endodontics, although a comparison of efficiency between the laser devices is not possible at present due to different study designs, materials, and equipment.

Short-wavelength infrared laser activates the auditory neurons: comparing the effect of 980 vs. 810 nm wavelength.

PubMed

Tian, Lan; Wang, Jingxuan; Wei, Ying; Lu, Jianren; Xu, Anting; Xia, Ming

2017-02-01

Research on auditory neural triggering by optical stimulus has been developed as an emerging technique to elicit the auditory neural response, which may provide an alternative method to the cochlear implants. However, most previous studies have been focused on using longer-wavelength near-infrared (>1800 nm) laser. The effect comparison of different laser wavelengths in short-wavelength infrared (SWIR) range on the auditory neural stimulation has not been previously explored. In this study, the pulsed 980- and 810-nm SWIR lasers were applied as optical stimuli to irradiate the auditory neurons in the cochlea of five deafened guinea pigs and the neural response under the two laser wavelengths was compared by recording the evoked optical auditory brainstem responses (OABRs). In addition, the effect of radiant exposure, laser pulse width, and threshold with the two laser wavelengths was further investigated and compared. The one-way analysis of variance (ANOVA) was used to analyze those data. Results showed that the OABR amplitude with the 980-nm laser is higher than the amplitude with the 810-nm laser under the same radiant exposure from 10 to 102 mJ/cm 2 . And the laser stimulation of 980 nm wavelength has lower threshold radiant exposure than the 810 nm wavelength at varied pulse duration in 20-500 μs range. Moreover, the 810-nm laser has a wider optimized pulse duration range than the 980-nm laser for the auditory neural stimulation.

Laser Application in Dentistry: Irradiation Effects of Nd:YAG 1064 nm and Diode 810 nm and 980 nm in Infected Root Canals—A Literature Overview

PubMed Central

Kuypers, Thorsten; Gutknecht, Norbert

2016-01-01

Objective. In endodontics, Nd:YAG laser (1064 nm) and diode laser (810 nm and 980 nm) devices are used to remove bacteria in infected teeth. A literature review was elaborated to compare and evaluate the advantages and disadvantages of using these lasers. Methods. Using combined search terms, eligible articles were retrieved from PubMed and printed journals. The initial search yielded 40 titles and 27 articles were assigned to full-text analysis. The studies were classified based upon laser source, laser energy level, duration/similarity of application, and initial and final bacterial count at a minimum of 20 prepared root canals. Part of the analysis was only reduced microorganisms and mechanically treated root canals upon preparation size of ISO 30. All studies were compared to evaluate the most favorable laser device for best results in endodontic therapy. Results. A total of 22 eligible studies were found regarding Nd:YAG laser 1064 nm. Four studies fulfilled all demanded criteria. Seven studies referring to the diode laser 980 nm were examined, although only one fulfilled all criteria. Eleven studies were found regarding the diode laser 810 nm, although only one study fulfilled all necessary criteria. Conclusions. Laser therapy is effective in endodontics, although a comparison of efficiency between the laser devices is not possible at present due to different study designs, materials, and equipment. PMID:27462611

Compact Laser-Based Sensors for Monitoring and Control of Gas Turbine Combustors

NASA Technical Reports Server (NTRS)

Hanson, Ronald K.; Jeffries, Jay B.

2003-01-01

Research is reported on the development of sensors for gas turbine combustor applications that measure real-time gas temperature using near-infrared water vapor absorption and concentration in the combustor exhaust of trace quantities of pollutant NO and CO using mid-infrared absorption. Gas temperature is extracted from the relative absorption strength of two near-infrared transitions of water vapor. From a survey of the water vapor absorption spectrum, two overtone transitions near 1800 nm were selected that can be rapidly scanned in wavelength by injection current tuning a single DFB diode laser. From the ratio of the absorbances on these selected transitions, a path-integrated gas temperature can be extracted in near-real time. Demonstration measurements with this new temperature sensor showed that combustor instabilities could be identified in the power spectrum of the temperature versus time record. These results suggest that this strategy is extremely promising for gas turbine combustor control applications. Measurements of the concentration of NO and CO in the combustor exhaust are demonstrated with mid-infrared transitions using thermo-electrically cooled, quantum cascade lasers operating near 5.26 and 4.62 microns respectively. Measurements of NO are performed in an insulated exhaust duct of a C2H4-air flame at temperatures of approximately 600 K. CO measurements are performed above a rich H2-air flame seeded with CO2 and cooled with excess N2 to 1150 K. Using a balanced ratiometric detection technique a sensitivity of 0.36 ppm-m was achieved for NO and 0.21 ppm-m for CO. Comparisons between measured and predicted water-vapor and CO2 interference are discussed. The mid-infrared laser quantum cascade laser technology is in its infancy; however, these measurements demonstrate the potential for pollutant monitoring in exhaust gases with mid-IR laser absorption.

Ferroelectric nanotraps for polar molecules

NASA Astrophysics Data System (ADS)

Dutta, Omjyoti; Giedke, G.

2018-02-01

We propose and analyze an electrostatic-optical nanoscale trap for cold diatomic polar molecules. The main ingredient of our proposal is a square array of ferroelectric nanorods with alternating polarization. We show that, in contrast to electrostatic traps using the linear Stark effect, a quadratic Stark potential supports long-lived trapped states. The molecules are kept at a fixed height from the nanorods by a standing-wave optical dipole trap. For the molecules and materials considered, we find nanotraps with trap frequency up to 1 MHz, ground-state width ˜20 nm with lattice periodicity of ˜200 nm . Analyzing the loss mechanisms due to nonadiabaticity, surface-induced radiative transitions, and laser-induced transitions, we show the existence of trapped states with lifetime ˜1 s , competitive with current traps created via optical mechanisms. As an application we extend our discussion to a one-dimensional (1D) array of nanotraps to simulate a long-range spin Hamiltonian in our structure.

Flame Characterization Using a Tunable Solid-State Laser with Direct UV Pumping

NASA Technical Reports Server (NTRS)

Kamal, Mohammed M.; Dubinskii, Mark A.; Misra, Prabhakar

1996-01-01

Tunable solid-state lasers with direct UV pumping, based on d-f transitions of rare earth ions incorporated in wide band-gap dielectric crystals, are reliable sources of laser radiation that are suitable for excitation of combustion-related free radicals. We have employed such a laser for analytical flame characterization utilizing Laser-Induced Fluorescence (LIF) techniques. LIF spectra of alkane-air flames (used for studying combustion processes under normal and microgravity conditions) excited in the region of the A-X (0,0) OH-absorption band have been recorded and found to be both temperature-sensitive and positionally-sensitive. In addition, also clearly noticeable was the sensitivity of the spectra to the specific wavelength used for data registration. The LiCAF:Ce laser shows good prospects for being able to cover the spectral region between 280 and 340 nm and therefore be used excitation of combustion-intermediates such as the hydroxyl OH, methoxy CH30 and methylthio CH3S radicals.

Cutting and skin-ablative properties of pulsed mid-infrared laser surgery.

PubMed

Kaufmann, R; Hartmann, A; Hibst, R

1994-02-01

Pulsed mid-infrared lasers allow a precise removal of soft tissues with only minimal thermal damage. To study the potential dermatosurgical usefulness of currently available systems at different wavelengths (2010-nm Thulium:YAG laser, 2100-nm Holmium:YAG laser, 2790-nm Erbium:YSGG laser, and 2940-nm Erbium:YAG laser) in vivo on pig skin. Immediate effects and wound healing of superficial laser-abrasions and incisions were compared with those of identical control lesions produced by dermabrasion, scalpel incisions, or laser surgery performed by a 1060-nm Nd:YAG and a 1060-nm CO2 laser (continuous and superpulsed mode). Best efficiency and least thermal injury was found for the pulsed Erbium:YAG laser, leading to ablative and incisional lesions comparable to those obtained by dermabrasion or superficial scalpel incisions, respectively. In contrast to other mid-infrared lasers tested, the 2940-nm Erbium:YAG laser thus provides a potential instrument for future applications in skin surgery, especially when aiming at a careful ablative removal of delicate superficial lesions with maximum sparing of adjacent tissue structures. However, in the purely incisional application mode pulsed mid-infrared lasers, though of potential usefulness in microsurgical indications (eg, surgery of the cornea), do not offer a suggestive alternative to simple scalpel surgery of the skin.

Lasers, extreme UV and soft X-ray

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nilsen, Joseph

2015-09-20

Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA)more » laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.« less

Absolute frequency measurement of a diode laser locked on a hyperfine component of 5S1/2-5D5/2 two-photon transitions of rubidium (lambda equals 778.1 nm, nu equals 385.3 THz)

NASA Astrophysics Data System (ADS)

Zondy, Jean-Jacques; Touahri, D.; Acef, Ouali; Hilico, L.; Abed, M.; Clairon, Andre; Millerioux, Yves P.; Felder, Raymond; de Beauvoir, Beatrice; Nez, Francois; Biraben, Francois; Julien, Lucile

1995-04-01

A frequency chain, derived from the one used to measure the absolute frequency ((nu) $= 473 THz) of the He-Ne/I2 optical standard, is currently being implemented in order to measure the frequency of a diode laser stabilized on the two-photon transition of rubidium vapor. The measurement scheme is based on the comparison of the frequency of this near-IR potential secondary standard to the 13th harmonic frequency of the R(12)-CO2/OsO4 LPTF secondary standard at (nu) equals 29.096 THz. Recent results on the frequency synthesis are reported, enabling the testing of long-term stability of this Rb-locked system with respect to the IR reference standard.

Nonradiative relaxation in tunable solid state laser crystals

NASA Technical Reports Server (NTRS)

Gayen, S. K.; Wang, W. B.; Petricevic, V.; Alfano, R. R.

1986-01-01

The characteristics of nonradiative transitions between the 4T2 and 2E excited states of trivalent-chromium-ion-activated ruby (containing 0.04 percent Cr2O3 by weight) and alexandrite (containing 0.4 at. percent chromium ion) laser crystals were studied using the technique described by Gayen et al. (1985). In this technique, a 527-nm pulse excites the 4T2 band of the Cr(3+), and the subsequent population kinetics among excited states is monitored by an IR picosecond probe pulse as a function of pump-probe delay. In ruby, a resolution-limited sharp rise in the excited state population was followed by a long-lifetime decay, leading to an upper limit of 7 ps for the 4T2-state nonradiative lifetime. In alexandrite, a longer rise time was followed by a multicomponent decay. A theoretical model is proposed for explaining the induced absorption and the transition dynamics observed in these crystals.

The effect of electromagnetically induced transparency in a potassium nanocell

NASA Astrophysics Data System (ADS)

Sargsyan, A.; Amiryan, A.; Leroy, C.; Vartanyan, T. A.; Sarkisyan, D.

2017-07-01

The effect of electromagnetically induced transparency (EIT) has been experimentally implemented for the first time for the (4 S 1/2-4 P 1/2-4 S 1/2) Λ-system of potassium atom levels in a nanocell with a 770-nm-thick column of atomic vapor. It is shown that, at such a small thickness of the vapor column, the EIT resonance can be observed only when the coupling-laser frequency is in exact resonance with the frequency of the corresponding atomic transition. The EIT resonance disappears even if the coupling-laser frequency differs slightly (by 50 MHz) from that of the corresponding atomic transition, which is due to the high thermal velocity of K atoms. The EIT resonance and related velocity selective optical pumping resonances caused by optical pumping (formed by the coupling) can be simultaneously recorded because of the small ( 462 MHz) hyperfine splitting of the lower 4 S 1/2 level.

Trivalent cerium coped crystals as tunable laser systems: two bad apples

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hamilton, D.S.

1985-01-01

The 5d-4f transitions of trivalent doped crystals have broad emission bands with large oscillator strengths and near unity quantum efficiency. These characteristics make cerium systems strong candidates for tunable solid state lasers. However, two such cerium crystals will probably never lase. The first is Ce/sup 3 +/:YAG where a strong excited state absorption quenches the lasing transition. Our recent measurements have indicated that the excited state absorption terminates in the YAG conduction band with a peak cross section of 1.0 x 10/sup -17/ cm/sup 2/ at 700 nm. Some of the general features of impurity ion to band spectra aremore » discussed. The second system is Ce/sup 3 +/:CaF/sub 2/ where a uv pump induced photochromic center is produced following excitation of the cerium ions. The initial measurements of cerium related transient absorptions in Ce/sup 3 +/:YLF are also presented.« less

Efficient 2.96 micron dysprosium-doped ZBLAN fibre laser pumped at 1.3 micron

NASA Astrophysics Data System (ADS)

Tsang, Yuen H.; El-Taher, Atalla E.; King, Terence A.; Chang, Kuang-Po; Jackson, Stuart D.

2006-04-01

Wavelengths around 1.15 μm, 1.3 μm and 1.7 μm can be used to pump Dy-doped ZBLAN fibre in order to generate ~3 μm with high efficiency. Previously the generation of 2.9 μm from the Dy-ZBLAN fibre was demonstrated by pumping with 1.1 μm Yb-silica fibre laser sources. The laser slope efficiency and lasing threshold demonstrated was about ~5% and ~1.78 W. In this investigation, the longer wavelength absorption band ( 6H 9/2 , 6F 11/2) centred at 1.3 μm of Dy 3+-doped ZBLAN is utilised and the lasing transition around ~3 μm takes places from 6H 13/2 --> 6H 15/2. With this pumping scheme the Stokes' efficiency is expected to be up to ~45%. A quasi-continuous wave Dy 3+-ZBLAN fibre laser pumped by a ~1.3 μm Nd:YAG laser and operating at 2.96 μm with a bandwidth (FWHM) of ~14 nm has been demonstrated. For a 60cm fibre length, a threshold of 0.5W and a slope efficiency of ~20% with respect to the absorbed pump power was observed. The overall pump absorption in the fibre was around 84%. The cavity reflectivities at 2.9 μm were 99% and 50%. The demonstrated slope efficiency was 45% of the Stokes' limit. The slope efficiency was around four times higher and the threshold around 3.6 times lower than the previous performance demonstrated by using the 1.1 μm Yb fibre laser pumping scheme. The higher performance achieved compared to the 1.1 μm pump scheme is due to the higher Stokes' limit, lower pump ESA losses and higher cavity reflectivity. About 590 cm -1 Raman Stokes shift has also detected by using 514.5 nm and 488 nm Ar ion laser as excitation pump sources.

Amplified spontaneous emission in N2 lasers: Saturation and bandwidth study

NASA Astrophysics Data System (ADS)

Hariri, A.; Sarikhani, S.

2014-05-01

A complete ASE analysis in a 3-level laser system based on the model of the geometrically dependent gain coefficient (GDGC) is presented. For the study, the photon density/intensity rate equation in the saturated and unsaturated conditions, along with reported experimental measurements on the ASE output energy and spectral bandwidth for N2-lasers were utilized. It was found that the GDGC model is able to explain the ASE output energy behavior and gain profiles correctly. In addition, the model was used to predict the spontaneous emission bandwidth Δν0 and consequently the stimulated emission cross-section for the C→B transition of nitrogen molecule at 337.1 nm. In this work, for example, Δν0 was found to be 766 GHz (2.9 Å) which is consistent with the earliest experimental observation on the ASE bandwidth reduction in a N2-laser as reported to be ~3. This is the first theoretical result that explains the spontaneous emission bandwidth which is different from the commonly used value of ~1 Å obtained from measurements of N2-lasers output spectra. The method was also applied for a filament N2 laser for the C→B transition produced in atmosphere, and a good consistency between the laboratory and filament lasers was obtained. Details of the calculations for this study are presented. The results obtained from 3-level systems confirm further the potential of applying the GDGC model for the ASE study in different laser systems and is unifying lasers of the same active medium.

Photoluminescence, thermoluminescence glow curve and emission characteristics of Y2O3:Er3+ nanophosphor.

PubMed

N J, Shivaramu; B N, Lakshminarasappa; K R, Nagabhushana; H C, Swart; Fouran, Singh

2018-01-15

Nanocrystalline Er 3+ doped Y 2 O 3 crystals were prepared by a sol gel technique. X-ray diffraction (XRD) patterns showed the cubic structure of Y 2 O 3 and the crystallite size was found to be ~25nm. Optical absorption showed absorption peaks at 454, 495 and 521nm. These peaks are attributed to the 4 F 3/2 + 4 F 5/2 , 4 F 7/2 and 2 H 11/2 + 4 S 3/2 transitions of Er 3+ . Under excitation at 378nm, the appearance of strong green (520-565nm) down conversion emission assigned to the ( 2 H 11/2, 4 S 3/2 )→ 4 I 15/2 transition and the feeble red (650-665nm) emission is assigned to the 4 F 9/2 → 4 I 15/2 transition. The color chromaticity coordinates showed emission in the green region. The strong green emission of Y 2 O 3 :Er 3+ nanophosphor may be useful for applications in solid compact laser devices. Thermoluminescence (TL) studies of γ-irradiated Y 2 O 3 :Er 3+ showed a prominent TL glow peak maximum at 383K along with a less intense shoulder peak at ~425K and a weak glow at 598K. TL emission peaks with maxima at 545, 490, 588 and 622nm for the doped sample were observed at a temperature of 383K and these emissions were due to defect related to the host material. TL kinetic parameters were calculated by a glow curve deconvolution (GCD) method and the obtained results are discussed in detail for their possible usage in high dose dosimetry. Copyright © 2017 Elsevier B.V. All rights reserved.

Photoluminescence, thermoluminescence glow curve and emission characteristics of Y2O3:Er3 + nanophosphor

NASA Astrophysics Data System (ADS)

N. J., Shivaramu; B. N., Lakshminarasappa; K. R., Nagabhushana; H. C., Swart; Fouran, Singh

2018-01-01

Nanocrystalline Er3 + doped Y2O3crystals were prepared by a sol gel technique. X-ray diffraction (XRD) patterns showed the cubic structure of Y2O3 and the crystallite size was found to be 25 nm. Optical absorption showed absorption peaks at 454, 495 and 521 nm. These peaks are attributed to the 4F3/2 + 4F5/2, 4F7/2 and 2H11/2 + 4S3/2 transitions of Er3 +. Under excitation at 378 nm, the appearance of strong green (520-565 nm) down conversion emission assigned to the (2H11/2,4S3/2) → 4I15/2 transition and the feeble red (650-665 nm) emission is assigned to the 4F9/2 → 4I15/2 transition. The color chromaticity coordinates showed emission in the green region. The strong green emission of Y2O3:Er3 + nanophosphor may be useful for applications in solid compact laser devices. Thermoluminescence (TL) studies of γ-irradiated Y2O3:Er3 + showed a prominent TL glow peak maximum at 383 K along with a less intense shoulder peak at 425 K and a weak glow at 598 K. TL emission peaks with maxima at 545, 490, 588 and 622 nm for the doped sample were observed at a temperature of 383 K and these emissions were due to defect related to the host material. TL kinetic parameters were calculated by a glow curve deconvolution (GCD) method and the obtained results are discussed in detail for their possible usage in high dose dosimetry.

Structural and optical investigation in Er3+ doped Y2MoO6 phosphors

NASA Astrophysics Data System (ADS)

Mondal, Manisha; Rai, Vineet Kumar

2018-05-01

The Er3+ doped Y2MoO6 phosphors have been structurally and optically characterized by X-ray Diffraction (XRD), Field emission scanning electron microscopy (FESEM), UV-Vis absorption spectroscopy and frequency upconversion (UC) emission studies. The crystal and the particles size are found to be ˜ 85 nm and ˜ 200 nm from XRD and FESEM analysis. The intense peak at ˜ 206 nm in the UV-Vis absorption spectroscopy is attributed due to the charge transfer transition between the Mo6+ and the O2- ions in the MoO4 group in the host molybdate. The frequency UC emission studies of the prepared phosphors under 980 nm diode laser excitation shows the intense UC emission in the 0.3 mol% concentrations for the Er3+ ions. In the UC emission spectra, the emission peaks at green (˜ 525 nm and ˜ 546 nm) and red (˜ 656 nm) bands are corresponding to the 2H11/2, 4S3/2 → 4I15/2 and 4F9/2 → 4I15/2 transitions of Er3+ ions. The mechanisms involved in the UC process have been explored with the help of energy level diagram. Moreover, the CIE point (0.31, 0.60) lie in the green colour region which indicates that the developed phosphor have suitable applications in NIR to visible upconverter and in making green light display devices.

Time delay and excitation mode induced tunable red/near-infrared to green emission ratio of Er doped BiOCl

NASA Astrophysics Data System (ADS)

Avram, Daniel; Florea, Mihaela; Tiseanu, Ion; Tiseanu, Carmen

2015-09-01

Herein, we report on the emission color tunability of Er doped BiOCl measured under up—conversion as well as x-ray excitation modes. The dependence of red (670 nm) to green emission (543 nm) ratio on Er concentration (1 and 5%), excitation wavelength into different (656.4, 802 and 976 nm) or across single Er absorption levels (965 ÷ 990 nm) and delay after the laser pulse (0.001 ÷ 1 ms) is discussed in terms of ground state absorption/excited state absorption and energy transfer up-conversion mechanisms. A first example of extended Er x-ray emission measured in the range of 500 to 1700 nm shows comparable emission intensities corresponding to 543 nm and 1500 nm based transitions. The present results together with our earlier report on the upconversion emission of Er doped BiOCl excited at 1500 nm, suggest that Er doped BiOCl may be considered an attractive system for optical and x-ray imaging applications.

A study of low threshold and high gain Nd3+ ions doped SiO2-B2O3-Na2CO3-NaF-CaF2 glasses for NIR laser applications

NASA Astrophysics Data System (ADS)

Megala, Rajesh; Gowthami, T.; John Sushma, N.; Kamala, S.; Deva Prasad Raju, B.

2018-05-01

Fluoroborosilicate glasses of composition 35SiO2-25B2O3-10Na2CO3-15NaF-15CaF2-xNd2O3 (where x = 0.1, 0.5. 1.0, 2.0 mol%) were prepared by melt quenching technique and various physical properties have been calculated. From the absorption spectra J-O Intensity parameters Ωλ (λ = 2, 4, 6) and radiative properties are evaluated by using J-O theory. The high values of Ω2 = 4.213 × 10-20 cm2, Ω4 = 5.345 × 10-20 cm2, Ω6 = 5.526 × 10-20 cm2 suggest that among the prepared glasses 0.5 mol% Nd glass is more asymmetric, more covalent and rigid in nature. The emission spectra were recorded with 808 nm laser as excitation source. The strong NIR emissions were observed at 876 nm, 1056 nm, 1328 nm corresponding to the transitions 4F3/2 → 4I9/2, 4F3/2 → 4I11/2, 4F3/2 → 4I13/2 respectively. Stimulated emission cross -section (σemi) and Gain bandwidth (σemi × Δλeff) were calculated. For 0.5 mol% Nd these values are found to be 3.30 × 10-20 cm2, 11 × 10-26 cm2. From the decay curve analysis the lifetime values for 4F3/2 level have been determined and these values are decreased with increase in Nd3+ ions concentration. These results may suggest that the prepared SBNCNd05 (Nd = 0.5 mol%) glass could be useful for 1056 nm laser applications.

Investigation of ASE and SRS effects on 1018nm short-wavelength Yb3+-doped fiber laser

NASA Astrophysics Data System (ADS)

Xie, Zhaoxin; Shi, Wei; Sheng, Quan; Fu, Shijie; Fang, Qiang; Zhang, Haiwei; Bai, Xiaolei; Shi, Guannan; Yao, Jianquan

2017-03-01

1018nm short wavelength Yb3+-doped fiber laser can be widely used for tandem-pumped fiber laser system in 1 μm regime because of its high brightness and low quantum defect (QD). In order to achieve 1018nm short wavelength Yb3+-doped fiber laser with high output power, a steady-state rate equations considering the amplified spontaneous emission (ASE) and Stimulated Raman Scattering (SRS) has been established. We theoretically analyzed the ASE and SRS effects in 1018nm short wavelength Yb3+-doped fiber laser and the simulation results show that the ASE is the main restriction rather than SRS for high power 1018nm short wavelength Yb3+-doped fiber laser, besides the high temperature of fiber is also the restriction for high output power. We use numerical solution of steady-state rate equations to discuss how to suppress ASE in 1018nm short wavelength fiber laser and how to achieve high power 1018nm short-wavelength fiber laser.

Assessment of femtosecond laser induced periodic surface structures on polymer films.

PubMed

Rebollar, Esther; Vázquez de Aldana, Javier R; Martín-Fabiani, Ignacio; Hernández, Margarita; Rueda, Daniel R; Ezquerra, Tiberio A; Domingo, Concepción; Moreno, Pablo; Castillejo, Marta

2013-07-21

In this work we present the formation of laser induced periodic surface structures (LIPSS) on spin-coated thin films of several model aromatic polymers including poly(ethylene terephthalate), poly(trimethylene terephthalate) and poly carbonate bis-phenol A upon irradiation with femtosecond pulses of 795 and 265 nm at fluences well below the ablation threshold. LIPSS are formed with period lengths similar to the laser wavelength and parallel to the direction of the laser polarization vector. Formation of LIPSS upon IR irradiation at 795 nm, a wavelength at which the polymers absorb weakly, contrasts with the absence of LIPSS in this spectral range upon irradiation with nanosecond pulses. Real and reciprocal space characterization of LIPSS obtained by Atomic Force Microscopy (AFM) and Grazing Incidence Small Angle X-ray Scattering (GISAXS), respectively, yields well correlated morphological information. Comparison of experimental and simulated GISAXS patterns suggests that LIPSS can be suitably described considering a quasi-one-dimensional paracrystalline lattice and that irradiation parameters have an influence on the order of such a lattice. Fluorescence measurements, after laser irradiation, provide indirect information about dynamics and structure of the polymer at the molecular level. Our results indicate that the LIPSS are formed by interference of the incident and surface scattered waves. As a result of this process, heating of the polymer surface above its glass transition temperature takes place enabling LIPSS formation.

Analysis of high-efficiency widely-tunable N-resonances in Cs vapor

NASA Astrophysics Data System (ADS)

Krasteva, A.; Gateva, S.; Tzvetkov, S.; Ghosh, P. N.; Sargsyan, A.; Cartaleva, S.

2018-03-01

The narrow-band coherent N-type resonance, promising for the development of advanced atomic clocks, can be considered as a type of three-photon resonance, where a two-photon Raman excitation is combined with a resonant optical pumping field. In this communication, we present an experimental study and a theoretical analysis related to three-photon, bi-chromatic excitation of Cs atomic vapor contained in an 8-mm long cell with 20 Torr of neon. If a coupling laser is fixed at a frequency that is lower by several GHz than the position of the absorption profile of the Fg = 4 set of transitions, and a probe laser is tuned over the D2 line (λ = 852 nm), a narrow high-contrast enhanced absorption N-resonance will be observed in the probe light profile, superimposed on the absorption profile of the Fg = 4 set of transitions. We present theoretical modeling aimed to clarify the processes behind the efficiency of the N-resonance preparation for different frequency positions of the coupling laser within the D2 line of Cs.

Laser ablation molecular isotopic spectroscopy (LAMIS) towards the determination of multivariate LODs via PLS calibration model of 10B and 11B Boric acid mixtures

NASA Astrophysics Data System (ADS)

Harris, C. D.; Profeta, Luisa T. M.; Akpovo, Codjo A.; Johnson, Lewis; Stowe, Ashley C.

2017-05-01

A calibration model was created to illustrate the detection capabilities of laser ablation molecular isotopic spectroscopy (LAMIS) discrimination in isotopic analysis. The sample set contained boric acid pellets that varied in isotopic concentrations of 10B and 11B. Each sample set was interrogated with a Q-switched Nd:YAG ablation laser operating at 532 nm. A minimum of four band heads of the β system B2∑ -> Χ2∑transitions were identified and verified with previous literature on BO molecular emission lines. Isotopic shifts were observed in the spectra for each transition and used as the predictors in the calibration model. The spectra along with their respective 10/11B isotopic ratios were analyzed using Partial Least Squares Regression (PLSR). An IUPAC novel approach for determining a multivariate Limit of Detection (LOD) interval was used to predict the detection of the desired isotopic ratios. The predicted multivariate LOD is dependent on the variation of the instrumental signal and other composites in the calibration model space.

Biomodulation of light on cells in laser surgery

NASA Astrophysics Data System (ADS)

Liu, Timon C.; Li, Yan; Duan, Rui; Cai, Xiongwei

2002-04-01

In laser surgery, it has been observed pulsed 532-nm laser can avoid postoperative purpura, but pulsed 585-nm, 595-nm or 600-nm lasers nonetheless cause purpura when they were used to treat port-wine stains; the XeCl excimer laser (308 nm) can safely and effectively clear psoriasis; both XeCl excimer laser and Ho:YAG laser were used in coronary interventions, but only former was approved by the FDA; open channels after ultraviolet (UV) laser treatment and closed channels with infrared (IR) lasers for transmyocardial laser revascularization; and so on. In this paper, the biological information model of low intensity laser (BIML) is extended to include UVA biomodulation and is used to understand these phenomena. Although the central intensity of the laser beam is so intense that it destroys the tissue, the edge intensity is so low that it can induce biomodulation. Our investigation showed that biomodulation of light on cells might play an important role in the long-term effects of laser surgery.

Investigation of the Fermi-Hubbard model with 6Li in an optical lattice

NASA Astrophysics Data System (ADS)

Hart, R. A.; Duarte, P. M.; Yang, T.-L.; Hulet, R. G.

2013-05-01

We present our results on investigation of the physics of the Fermi-Hubbard model using an ultracold gas of 6Li loaded into an optical lattice. We use all-optical methods to efficiently cool and load the lattice beginning with laser cooling on the 2S1 / 2 --> 2P3 / 2 transition and then further cooling using the narrow 2S1 / 2 --> 3P3 / 2 transition to T ~ 59 μK. The second stage of laser cooling greatly enhances loading to an optical dipole trap where a two spin state mixture of atoms is evaporatively cooled to degeneracy. We then adiabatically load ~106 degenerate fermions into a 3D optical lattice formed by three orthogonal standing waves of 1064 nm light. Overlapped with each of the three lattice beams is a non-retroreflected beam at 532 nm. This light cancels the harmonic trapping caused by the lattice beams, which extends the number of lattice sites over which a Néel phase can exist and may allow evaporative cooling in the lattice. By using Bragg scattering of light, we investigate the possibility of observing long-range antiferromagnetic ordering of spins in the lattice. Supported by NSF, ONR, DARPA, and the Welch Foundation.

The effect of bleaching gel and (940 nm and 980 nm) diode lasers photoactivation on intrapulpal temperature and teeth whitening efficiency.

PubMed

Al-Karadaghi, Tamara S; Al-Saedi, Asmaa A; Al-Maliky, Mohammed A; Mahmood, Ali S

2016-12-01

This in vitro study aimed to investigate the whitening efficacy of 940 nm and 980 nm diode laser photoactivation in tooth bleaching by analysing pulp chamber temperature, as well as the change in tooth colour. Root canals of thirty extracted human lower premolars were prepared. Laserwhite* 20 bleaching agent containing 38% of hydrogen peroxide was photoactivated with 7 W output power of 940 nm and 980 nm diode lasers for 120 s. Bleaching gel reduced 27-29% of the temperature from reaching the pulp chamber. For shade assessment, only the groups photoactivated using diode lasers showed statistically significant differences from control group P < 0.001. Within the studied parameters, both 940 nm and 980 nm diode lasers produced a safe pulp temperature increase. Diode laser photoactivation of bleaching gel resulted in more efficient teeth whitening. Photoactivation with 940 nm diode laser yielded the highest change in colour with only minor increase in pulp chamber temperature. © 2016 Australian Society of Endodontology Inc.

On The Stark Shift of Ar II 472.68 nm Spectral Line

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mijatovic, Z.; Gajo, T.; Vujicic, B.

The Stark shift of Ar II 472.68 nm (transition 4s2P - 4p2D deg. ) spectral lines emitted from T-tube plasmas was considered. The electron density ranged from (1.63-2.2){center_dot}1023 m-3 and was determined using laser interferometry. The plasma temperature, derived from the Gaussian part of recorded line profiles was found to be in the range (15000-43300) K. Experimental shifts were compared to theoretical values obtained from the semiempirical formula [M. S. Dimitrijevic and N. Konjevic, J. Quant. Spectrosc. Radiat. Transfer 24, 451 (1980)]. This comparison showed good agreement between experimental results and theory.

Micro ion frequency standard

NASA Astrophysics Data System (ADS)

Schwindt, Peter D. D.; Jau, Yuan-Yu; Partner, Heather; Serkland, Darwin K.; Boye, Robert; Fang, Lu; Casias, Adrian; Manginell, Ronald P.; Moorman, Matthew; Prestage, John; Yu, Nan

2011-06-01

We are developing a highly miniaturized trapped ion clock to probe the 12.6 GHz hyperfine transition in the 171Yb+ ion. The clock development is being funded by the Integrated Micro Primary Atomic Clock Technology (IMPACT) program from DARPA where the stated goals are to develop a clock that consumes 50 mW of power, has a size of 5 cm3, and has a long-term frequency stability of 10-14 at one month. One of the significant challenges will be to develop miniature single-frequency lasers at 369 nm and 935 nm and the optical systems to deliver light to the ions and to collect ion fluorescence on a detector.

Observations of z-dependent microbunching harmonic intensities using COTR in a SASE FEL.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lumpkin, A. H.; Biedron, S. G.; Dejus, R. J.

The nonlinear generation of harmonics in a self-amplified spontaneous emission (SASE) free-electron laser (FEL) continues to be of interest. Complementary to such studies is the search for information on the electron beam microbunching harmonic components, which are revealed by coherent optical transition radiation (COTR) experiments. An initial z-dependent set of data has been obtained with the fundamental at 530 nm and the second harmonic at 265 nm. The latter data were collected after every other undulator in a nine-undulator string. These results are compared to estimates based on GINGER and an analytical model for nonlinear harmonic generation.

All-fibre ytterbium laser tunable within 45 nm

DOE Office of Scientific and Technical Information (OSTI.GOV)

Abdullina, S R; Babin, S A; Vlasov, A A

2007-12-31

A tunable ytterbium-doped fibre laser is fabricated. The laser is tuned by using a tunable fibre Bragg grating (FBG) as a selecting intracavity element. The laser is tunable within 45 nm (from 1063 to 1108 nm) and emits {approx}6 W in the line of width {approx}0.15 nm, the output power and linewidth being virtually invariable within the tuning range. The method is proposed for synchronous tuning the highly reflecting and output FBGs, and a tunable ytterbium all-fibre laser is built. (lasers)

The laser-diode-excited 5 d-4 f luminescence of Ce3+ and Pr3+ ions embedded into a BaR2F8 matrix

NASA Astrophysics Data System (ADS)

Pushkar', A. A.; Uvarova, T. V.; Kozlova, N. S.; Kuznetsov, S. Yu.; Uvarova, A. G.

2013-06-01

We show the possibility of obtaining UV luminescence from 5 d-4 f transitions of rare-earth ions in the BaY2F8: (Yb3+, Pr3+, Ce3+) crystal under upconversion excitation by standard laser diodes with lasing wavelengths of 960, 808, and 840 nm. Various upconversion mechanisms of pumping for populating the higher-lying energy levels of the active ions, as well as methods of adaptation of the active medium BaY2F8: (Yb3+, Pr3+, Ce3+) to these mechanisms, are considered.

Multi-species detection using multi-mode absorption spectroscopy (MUMAS)

NASA Astrophysics Data System (ADS)

Northern, J. H.; Thompson, A. W. J.; Hamilton, M. L.; Ewart, P.

2013-06-01

The detection of multiple species using a single laser and single detector employing multi-mode absorption spectroscopy (MUMAS) is reported. An in-house constructed, diode-pumped, Er:Yb:glass micro-laser operating at 1,565 nm with 10 modes separated by 18 GHz was used to record MUMAS signals in a gas mixture containing C2H2, N2O and CO. The components of the mixture were detected simultaneously by identifying multiple transitions in each of the species. By using temperature- and pressure-dependent modelled spectral fits to the data, partial pressures of each species in the mixture were determined with an uncertainty of ±2 %.

Renal denervation using focused infrared fiber lasers: a potential treatment for hypertension.

PubMed

Alexander, Vinay V; Shi, Zhennan; Iftekher, Fariha; Welsh, Michael J; Gurm, Hitinder S; Rising, Gail; Yanovich, Amber; Walacavage, Kim; Islam, Mohammed N

2014-11-01

Renal denervation has recently become of great interest as a potential treatment for resistant hypertension. Denervation techniques using radio frequency (RF) or ultrasound energy sources have already been explored in literature. In this study, we investigate the use of lasers as a potential energy source for renal denervation. In vitro studies are performed in porcine/ovine renal arteries with focused laser beams at 980 nm, 1210 nm, and 1700 nm to study the ability to damage renal nerves without causing injury to non-target tissue structures like the endothelium. Then, a 980 nm laser catheter prototype is built and used to demonstrate in vivo renal denervation in ovine renal arteries. This study utilizes fiber coupled infrared lasers at 980 nm, 1210 nm, and 1700 nm. In vitro laser denervation studies at 980 nm are performed in both porcine and ovine renal arteries to study the ability of focused laser beams to damage renal nerves without injuring the endothelium. In vitro studies using lasers close to the lipid absorption lines at 1210 nm and 1700 nm are also performed in porcine renal arteries to study the possibility of selectively damaging the renal nerves by targeting the lipid myelin sheaths surrounding the nerves. Then, a laser catheter prototype is designed and built for in vivo renal denervation in ovine renal arteries using the 980 nm laser (powers ranging from 2 to 4 W, 5 seconds per exposure). Histochemical evaluations of the frozen sections are performed using methylthiazolyldiphenyl-tetrazolium bromide (MTT) assay. Histochemical analysis of in vitro laser treatments at 980 nm in porcine and ovine renal arteries show clear evidence of laser-induced renal nerve damage without injury to the endothelium and part of the media. No evidence of selective nerve damage is observed using the 1210 nm and 1700 nm lasers with the current treatment parameters. Histochemical analysis of in vivo laser treatments in ovine renal arteries using a focused 980 nm laser show clear evidence of renal nerve damage with depths of damage extending > 1.5 mm from the artery wall. Sections with laser-induced damage to the media/adventitia at depths of > 1 mm without injury to the endothelium are also observed. We demonstrate the use of focused lasers as an attractive energy source for causing renal nerve damage without injury to the artery wall and thus, may have potential therapeutic applications for conditions such as resistant hypertension, where renal denervation has been shown to be a promising form of treatment. © 2014 Wiley Periodicals, Inc.

Effects of optical dopants and laser wavelength on atom probe tomography analyses of borosilicate glasses

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lu, Xiaonan; Schreiber, Daniel K.; Neeway, James J.

Atom probe tomography (APT) is a novel analytical microscopy method that provides three dimensional elemental mapping with sub-nanometer spatial resolution and has only recently been applied to insulating glass and ceramic samples. In this paper, we have studied the influence of the optical absorption in glass samples on APT characterization by introducing different transition metal optical dopants to a model borosilicate nuclear waste glass (international simple glass). A systematic comparison is presented of the glass optical properties and the resulting APT data quality in terms of compositional accuracy and the mass spectra quality for two APT systems: one with amore » green laser (532 nm, LEAP 3000X HR) and one with a UV laser (355 nm, LEAP 4000X HR). These data were also compared to the study of a more complex borosilicate glass (SON68). The results show that the analysis data quality such as compositional accuracy and total ions collected, was clearly linked to optical absorption when using a green laser, while for the UV laser optical doping aided in improving data yield but did not have a significant effect on compositional accuracy. Comparisons of data between the LEAP systems suggest that the smaller laser spot size of the LEAP 4000X HR played a more critical role for optimum performance than the optical dopants themselves. The smaller spot size resulted in more accurate composition measurements due to a reduced background level independent of the material’s optical properties.« less

Prospective study of the 532 nm laser (KTP) versus diode laser 980 nm in the resection of hyperplastic lesions of the oral cavity

PubMed Central

Bargiela-Pérez, Patricia; González-Merchán, Jorge; Díaz-Sánchez, Rosa; Serrera-Figallo, Maria-Angeles; Volland, Gerd; Joergens, Martin; Gutiérrez-Pérez, Jose-Luis

2018-01-01

Background The aim of this study is to evaluate the resection of hyperplastic lesions on the buccal mucosa comparing the 532nm laser (KTP), versus diode 980nm laser, considering pain, scarring, inflammation and drug consumption that occurred postoperatively with each lasers. Material and Methods A prospective study of consecutive series of 20 patients in two groups that presents hyperplastic lesions on the buccal mucosa. The choice of the KTP laser or diode 980nm laser for the surgery was made randomly. The power used was 1.5W in both groups in a continuous wave mode with a 320 μm optical fiber. Parameters of pain, scarring, inflammation and consumption of drugs were recorded by a Numerical Rating Scale and evaluated postoperatively. These recordings were made the day of the surgery, 24 hours after, 14 and 28 days after. Results Pain and inflammation was light - moderate. The consumption of paracetamol was somewhat higher in the diode 980nm laser versus the KTP laser after 24 hours, although data was not statistically significant; significant differences were found after 28 days in regards to pain (p = 0.023) and inflammation (p = 0.023), but always in the absence parameter so we find no pain in both lasers. Scarring in the two types of laser showed no differences along the visits, with not detected scar retractable. Conclusions Although there is a slight histological difference regarding the KTP laser in the oral soft tissues for clinical use, both wavelengths are very suitable for excision of oral fibroma. Key words:Laser surgery, Laser therapy, oral surgery, soft tissue, 980 nm diode laser, 532 nm KTP laser. PMID:29274158

Study of the laser-induced decomposition of energetic materials at static high-pressure by time-resolved absorption spectroscopy

NASA Astrophysics Data System (ADS)

Hebert, Philippe; Saint-Amans, Charles

2013-06-01

A detailed description of the reaction rates and mechanisms occurring in shock-induced decomposition of condensed explosives is very important to improve the predictive capabilities of shock-to-detonation transition models. However, direct measurements of such experimental data are difficult to perform during detonation experiments. By coupling pulsed laser ignition of an explosive in a diamond anvil cell (DAC) with time-resolved streak camera recording of transmitted light, it is possible to make direct observations of deflagration phenomena at detonation pressure. We have developed an experimental set-up that allows combustion front propagation rates and time-resolved absorption spectroscopy measurements. The decomposition reactions are initiated using a nanosecond YAG laser and their kinetics is followed by time-resolved absorption spectroscopy. The results obtained for two explosives, nitromethane (NM) and HMX are presented in this paper. For NM, a change in reactivity is clearly seen around 25 GPa. Below this pressure, the reaction products are essentially carbon residues whereas at higher pressure, a transient absorption feature is first observed and is followed by the formation of a white amorphous product. For HMX, the evolution of the absorption as a function of time indicates a multi-step reaction mechanism which is found to depend on both the initial pressure and the laser fluence.

Simulations of laser-driven ion acceleration from a thin CH target

NASA Astrophysics Data System (ADS)

Park, Jaehong; Bulanov, Stepan; Ji, Qing; Steinke, Sven; Treffert, Franziska; Vay, Jean-Luc; Schenkel, Thomas; Esarey, Eric; Leemans, Wim; Vincenti, Henri

2017-10-01

2D and 3D computer simulations of laser driven ion acceleration from a thin CH foil using code WARP were performed. As the foil thickness varies from a few nm to μm, the simulations confirm that the acceleration mechanism transitions from the RPA (radiation pressure acceleration) to the TNSA (target normal sheath acceleration). In the TNSA regime, with the CH target thickness of 1 μ m and a pre-plasma ahead of the target, the simulations show the production of the collimated proton beam with the maximum energy of about 10 MeV. This agrees with the experimental results obtained at the BELLA laser facility (I 5 × 18 W / cm2 , λ = 800 nm). Furthermore, the maximum proton energy dependence on different setups of the initialization, i.e., different angles of the laser incidence from the target normal axis, different gradient scales and distributions of the pre-plasma, was explored. This work was supported by LDRD funding from LBNL, provided by the U.S. DOE under Contract No. DE-AC02-05CH11231, and used resources of the NERSC, a DOE office of Science User Facility supported by the U.S. DOE under Contract No. DE-AC02-05CH11231.

Abnormal photothermal effect of laser radiation on highly defect oxide bronze nanoparticles under the sub-threshold excitation of absorption

NASA Astrophysics Data System (ADS)

Gulyaev, P.; Kotvanova, M.; Omelchenko, A.

2017-05-01

The mechanism of abnormal photo-thermal effect of laser radiation on nanoparticles of oxide bronzes has been proposed in this paper. The basic features of the observed effect are: a) sub-threshold absorption of laser radiation by the excitation of donor-like levels formed in the energy gap due to superficial defects of the oxide bronze nano-crystals; b) an interband radiationless transition of energy of excitation on deep triplet levels and c) consequent recombination occurring at the plasmon absorption. K or Na atoms thermally intercalated to the octahedral crystal structure of TiO2 in the wave SHS combustion generate acceptor levels in the gap. The prepared oxide bronzes of the non-stoichiometric composition NaxTiO2 and KxTiO2 were examined by high resolution TEM, and then grinded in a planetary mill with powerful dispersion energy density up to 4000 J/g. This made it possible to obtain nanoparticles about 50 nm with high surface defect density (1017-1019 cm-2 at a depth of 10 nm). High photo-thermal effect of laser radiation on the defect nanocrystals observed after its impregnation into cartilaginous tissue exceeds 7 times in comparison with the intact ones.

Ocular damage effects from 1338-nm pulsed laser radiation in a rabbit eye model

PubMed Central

Jiao, Luguang; Wang, Jiarui; Jing, Xiaomin; Chen, Hongxia; Yang, Zaifu

2017-01-01

The ocular damage effects induced by transitional near-infrared (NIR) lasers have been investigated for years. However, no retinal damage thresholds are determined in a wide interval between 0.65 ms and 80 ms, and a definite relationship between corneal damage threshold and spot size cannot be drawn from existing data points. In this paper, the in-vivo corneal damage thresholds (ED50s) were determined in New Zealand white rabbits for a single 5 ms pulse at the wavelength of 1338 nm for spot sizes from 0.28 mm to 3.55 mm. Meanwhile, the retinal damage threshold for this laser was determined in chinchilla grey rabbits under the condition that the beam was collimated, and the incident corneal spot diameter was 5.0 mm. The corneal ED50s given in terms of the corneal radiant exposure for spot diameters of 0.28, 0.94, 1.91, and 3.55 mm were 70.3, 35.6, 29.6 and 30.3 J/cm2, respectively. The retinal ED50 given in terms of total intraocular energy (TIE) was 0.904 J. The most sensitive ocular tissue to this laser changed from the cornea to retina with the increase of spot size. PMID:28663903

Optically controlled polarizer using a ladder transition for high speed Stokesmetric Imaging and Quantum Zeno Effect based optical logic.

PubMed

Krishnamurthy, Subramanian; Wang, Y; Tu, Y; Tseng, S; Shahriar, M S

2013-10-21

We demonstrate an optically controlled polarizer at ~1323 nm using a ladder transition in a Rb vapor cell. The lower leg of the 5S(1/2),F = 1->5P(1/2),F = 1,2->6S(1/2),F = 1,2 transitions is excited by a Ti:Sapphire laser locked to a saturated absorption signal, representing the control beam. A tunable fiber laser at ~1323 nm is used to excite the upper leg of the transitions, representing the signal beam. When the control beam is linearly polarized, it produces an excitation of the intermediate level with a particular orientation of the angular momentum. Under ideal conditions, this orientation is transparent to the signal beam if it has the same polarization as the control beam and is absorbed when it is polarized orthogonally. We also present numerical simulations of the system using a comprehensive model which incorporates all the relevant Zeeman sub-levels in the system, and identify means to improve the performance of the polarizer. A novel algorithm to compute the evolution of large scale quantum system enabled us to perform this computation, which may have been considered too cumbersome to carry out previously. We describe how such a polarizer may serve as a key component for high-speed Stokesmetric imaging. We also show how such a polarizer, combined with an optically controlled waveplate, recently demonstrated by us, can be used to realize a high speed optical logic gate by making use of the Quantum Zeno Effect. Finally, we describe how such a logic gate can be realized at an ultra-low power level using a tapered nanofiber embedded in a vapor cell.

Wavelength dependence on the forensic analysis of glass by nanosecond 266 nm and 1064 nm laser induced breakdown spectroscopy

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cahoon, Erica M.; Almirall, Jose R.

Laser induced breakdown spectroscopy can be used for the chemical characterization of glass to provide evidence of an association between a fragment found at a crime scene to a source of glass of known origin. Two different laser irradiances, 266 nm and 1064 nm, were used to conduct qualitative and quantitative analysis of glass standards. Single-pulse and double-pulse configurations and lens-to-sample-distance settings were optimized to yield the best laser-glass coupling. Laser energy and acquisition timing delays were also optimized to result in the highest signal-to-noise ratio corresponding to the highest precision and accuracy. The crater morphology was examined and themore » mass removed was calculated for both the 266 nm and 1064 nm irradiations. The analytical figures of merit suggest that the 266 nm and 1064 nm wavelengths are capable of good performance for the forensic chemical characterization of glass. The results presented here suggest that the 266 nm laser produces a better laser-glass matrix coupling, resulting in a better stoichiometric representation of the glass sample. The 266 nm irradiance is therefore recommended for the forensic analysis and comparison of glass samples.« less

Surface microstructure and chemistry of polyimide by single pulse ablation of picosecond laser

NASA Astrophysics Data System (ADS)

Du, Qifeng; Chen, Ting; Liu, Jianguo; Zeng, Xiaoyan

2018-03-01

Polyimide (PI) surface was ablated by the single pulse of picosecond laser, and the effects of laser wavelength (λ= 355 nm and 1064 nm) and fluence on surface microstructure and chemistry were explored. Scanning electron microscopy (SEM) analysis found that different surface microstructures, i.e., the concave of concentric ring and the convex of porous circular disk, were generated by 355 nm and 1064 nm picosecond laser ablation, respectively. X-ray photoelectron spectroscopy (XPS) characterization indicated that due to the high peak energy density of picosecond laser, oxygen and nitrogen from the ambient were incorporated into the PI surface mainly in the form of Cdbnd O and Csbnd Nsbnd C groups. Thus, both of the O/C and N/C atomic content ratios increased, but the increase caused by 1064 nm wavelength laser was larger. It inferred that the differences of PI surface microstructures and chemistry resulted from different laser parameters were related to different laser-matter interaction effects. For 355 nm picosecond laser, no obvious thermal features were observed and the probable ablation process of PI was mainly governed by photochemical effect; while for 1064 nm picosecond laser, obvious thermal feature appeared and photothermal effect was thought to be dominant.

303 nm continuous wave ultraviolet laser generated by intracavity frequency-doubling of diode-pumped Pr3+:LiYF4 laser

NASA Astrophysics Data System (ADS)

Zhu, Pengfei; Zhang, Chaomin; Zhu, Kun; Ping, Yunxia; Song, Pei; Sun, Xiaohui; Wang, Fuxin; Yao, Yi

2018-03-01

We demonstrate an efficient and compact ultraviolet laser at 303 nm generated by intracavity frequency doubling of a continuous wave (CW) laser diode-pumped Pr3+:YLiF4 laser at 607 nm. A cesium lithium borate (CLBO) crystal, cut for critical type I phase matching at room temperature, is used for second-harmonic generation (SHG) of the fundamental laser. By using an InGaN laser diode array emitting at 444.3 nm with a maximum incident power of 10 W, as high as 68 mW of CW output power at 303 nm is achieved. The output power stability in 4 h is better than 2.85%. To the best of our knowledge, this is high efficient UV laser generated by frequency doubling of an InGaN laser diode array pumped Pr3+:YLiF4 laser.

Diode laser-induced tissue effects: in vitro tissue model study and in vivo evaluation of wound healing following non-contact application.

PubMed

Havel, Miriam; Betz, Christian S; Leunig, Andreas; Sroka, Ronald

2014-08-01

The basic difference between the various common medical laser systems is the wavelength of the emitted light, leading to altered light-tissue interactions due to the optical parameters of the tissue. This study examines laser induced tissue effects in an in vitro tissue model using 1,470 nm diode laser compared to our standard practice for endonasal applications (940 nm diode laser) under standardised and reproducible conditions. Additionally, in vivo induced tissue effects following non-contact application with focus on mucosal healing were investigated in a controlled intra-individual design in patients treated for hypertrophy of nasal turbinate. A certified diode laser system emitting the light of λ = 1470 nm was evaluated with regards to its tissue effects (ablation, coagulation) in an in vitro setup on porcine liver and turkey muscle tissue model. To achieve comparable macroscopic tissue effects the laser fibres (600 µm core diameter) were fixed to a computer controlled stepper motor and the laser light was applied in a reproducible procedure under constant conditions. For the in vivo evaluation, 20 patients with nasal obstruction due to hyperplasia of inferior nasal turbinates were included in this prospective randomised double-blinded comparative trial. The endoscopic controlled endonasal application of λ = 1470 nm on the one and λ = 940 nm on the other side, both in 'non-contact' mode, was carried out as an outpatient procedure under local anaesthesia. The postoperative wound healing process (mucosal swelling, scab formation, bleeding, infection) was endoscopically documented and assessed by an independent physician. In the experimental setup, the 1,470 nm laser diode system proved to be efficient in inducing tissue effects in non-contact mode with a reduced energy factor of 5-10 for highly perfused liver tissue to 10-20 for muscle tissue as compared to the 940 nm diode laser system. In the in vivo evaluation scab formation following laser surgery as assessed clinically on endonasal endoscopy was significantly reduced on 1,470 nm treated site compared to 940 nm diode laser treated site. Diode laser system (1,470 nm) induces efficient tissue effects compared to 940 nm diode laser system as shown in the tissue model experiment. From the clinical point of view, the healing process following non-contact diode laser application revealed to be improved using 1,470 nm diode laser compared to our standard diode laser practise with 940 nm. © 2014 Wiley Periodicals, Inc.

Photodynamic impact induces ischemic tolerance in models in vivo and in vitro

NASA Astrophysics Data System (ADS)

Demyanenko, Svetlana; Sharifulina, Svetlana; Berezhnaya, Elena; Kovaleva, Vera; Neginskaya, Maria; Zhukovskaya, Ludmila

2016-04-01

Ischemic tolerance determines resistance to lethal ischemia gained by a prior sublethal stimulus (i.e., preconditioning). We reproduced this effect in two variants. In vitro the preliminary short (5 s) photodynamic treatment (PDT) (photosensitizer Photosens, 10 nM, 30 min preincubation; laser: 670 nm, 100 mW/cm2) significantly reduced the necrosis of neurons and glial cells in the isolated crayfish stretch receptor, which was caused by following 30-min PDT by 66% and 46%, respectively. In vivo PDT of the rat cerebral cortex with hydrophilic photosensitizer Rose Bengal (i.v. administration, laser irradiation: 532 nm, 60 mW/cm2, 3 mm beam diameter, 30 min) caused occlusion of small brain vessels and local photothrombotic infarct (PTI). It is a model of ischemic stroke. Cerebral tissue edema and global necrosis of neurons and glial cells occurred in the infarction core, which was surrounded by a 1.5 mm transition zone, penumbra. The maximal pericellular edema, hypo- and hyperchromia of neurons were observed in penumbra 24 h after PTI. The repeated laser irradiation of the contralateral cerebral cortex also caused PTI but lesser as compared with single PDT. Preliminary unilateral PTI provided ischemic tolerance: at 14 day after second exposure the PTI volume significantly decreased by 24% than in the case of a single exposure. Sensorimotor deficits in PDT-treated rats was registered using the behavioral tests. The preliminary PTI caused the preconditioning effect.

Design and analysis of InN - In0.25Ga0.75N single quantum well laser for short distance communication wavelength

NASA Astrophysics Data System (ADS)

Polash, Md. Mobarak Hossain; Alam, M. Shah; Biswas, Saumya

2018-03-01

A single quantum well semiconductor laser based on wurtzite-nitride is designed and analyzed for short distance communication wavelength (at around 1300 nm). The laser structure has 12 Å well layer of InN, 15 Å barrier layer of In0.25Ga0.75N, and 54 Å separate confinement heterostructure layer of GaN. To calculate the electronic characteristics of the structure, a self-consistent method is used where Hamiltonian with effective mass approximation is solved for conduction band while six-bands Hamiltonian matrix with k · p formalism including the polarization effect, valence-band mixing effect, and strain effect is solved for valence band. The interband optical transition elements, optical gain, differential gain, radiative current density, spontaneous emission rate, and threshold characteristics have been calculated. The wave function overlap integral is found to be 45.93% for TE-polarized structure. Also, the spontaneous emission rate is found to be 6.57 × 1027 s - 1 cm - 3 eV - 1 at 1288.21 nm with the carrier density of 5 × 1019 cm - 3. Furthermore, the radiative current density and the radiative recombination rate are found to be 121.92 A cm - 2 and 6.35 × 1027 s - 1 cm - 3, respectively, while the TE-polarized optical gain of the structure is 3872.1 cm - 1 at 1301.7 nm.

Measurements of Effective Schottky Barrier in Inverse Extraordinary Optoconductance Structures

NASA Astrophysics Data System (ADS)

Tran, L. C.; Werner, F. M.; Solin, S. A.; Gilbertson, Adam; Cohen, L. F.

2013-03-01

Individually addressable optical sensors with dimensions as low as 250nm, fabricated from metal semiconductor hybrid structures (MSH) of AuTi-GaAs Schottky interfaces, display a transition from resistance decreasing with intensity in micron-scale sensors (Extraordinary Optoconductance, EOC) to resistance increasing with intensity in nano-scale sensors (Inverse Extraordinary Optoconductance I-EOC). I-EOC is attributed to a ballistic to diffusive crossover with the introduction of photo-induced carriers and gives rise to resistance changes of up to 9462% in 250nm devices. We characterize the photo-dependence of the effective Schottky barrier in EOC/I-EOC structures by the open circuit voltage and reverse bias resistance. Under illumination by a 5 mW, 632.8 nm HeNe laser, the barrier is negligible and the Ti-GaAs interface becomes Ohmic. Comparing the behavior of two devices, one with leads exposed, another with leads covered by an opaque epoxy, the variation in Voc with the position of the laser can be attributed to a photovoltaic effect of the lead metal and bulk GaAs. The resistance is unaffected by the photovoltaic offset of the leads, as indicated by the radial symmetry of 2-D resistance maps obtained by rastering a laser across EOC/IEOC devices. SAS has a financial interest in PixelEXX, a start-up company whose mission is to market imaging arrays.

Development of infrared sensors using energy transfer/energy upconversion processes: Study of laser excited fluorescence in rare Earth ion doped crystals

NASA Technical Reports Server (NTRS)

Nash-Stevenson, S. K.; Reddy, B. R.; Venkateswarlu, P.

1994-01-01

A summary is presented of the spectroscopic study of three systems: LaF3:Ho(3+), LaF3:Er(3+) and CaF2:Nd(3+). When the D levels of Ho(3+) in LaF3 were resonantly excited with a laser beam of 640 nm, upconverted emissions were detected from J (416 nm), F (485 nm), and E (546 nm) levels. Energy upconverted emissions were also observed from F and E levels of Ho(3+) when the material was excited with an 800 nm near infrared laser. When the D levels of Er(3+) in LaF3 were resonantly excited with a laser beam of 637 nm, upconverted emissions were detected from the E (540 nm) and P (320, 400, and 468 nm) levels. Energy upconverted emissions were also observed from F, E, and D levels of Er(3+) when the material was resonantly excited with an 804 nm near infrared laser. When the D levels of Nd(3+) in CaF2 were resonantly excited with a laser beam of 577 nm, upconverted emissions were detected from the L (360 and 382 nm), K (418 nm), and I (432 nm) levels. Very weak upconverted emissions were detected when this system was irradiated with a near infrared laser. The numbers in parentheses are the wavelengths of the emissions.

Lifetime behavior of laser diodes with highly strained InGaAs QWs and emission wavelength between 1120 nm and 1180 nm

NASA Astrophysics Data System (ADS)

Bugge, F.; Bege, R.; Blume, G.; Feise, D.; Sumpf, B.; Werner, N.; Zeimer, U.; Paschke, K.; Weyers, M.

2018-06-01

Highly strained InxGa1-xAs QWs are commonly used for laser diodes in the wavelength range beyond 1100 nm, but they suffer from strain induced formation of defects. The effect of different laser structures and different laser layouts on the aging behavior was investigated. If grown and processed under optimized conditions, laser diodes emitting at 1120 nm, 1156 nm and 1180 nm have lifetimes of several 1000 h up to more than 20,000 h in dependence on structure or indium content. Laser diodes with three different emission wavelength were mounted in a microoptical bench with a second harmonic generation crystal. From these benches laser emission in the green-yellow spectral range with more than 800 mW output power was obtained.

Laser action in chromium-activated forsterite for near infrared excitation

NASA Technical Reports Server (NTRS)

Petricevic, V.; Gayen, S. K.; Alfano, R. R.

1988-01-01

This paper reports on laser action in chromium-doped forsterite (Cr:Mg2SiO4) for 1064-nm excitation of the crystal's double-hump absorption band spanning the 850-1200-nm wavelength range. The cavity arrangement used for obtaining laser action in Cr:Mg2SiO2 was similar to that described by Petricevic et al. (1988). The fundamental and second harmonic emissions from a Q-switched Nd:YAG laser operating at a 10-Hz repetition rate were used for excitation of the NIR and visible bands, respectively. Pulsed laser action was readily observed for both the 1064-nm and 532-nm pumping at or above the respective thresholds. The laser parameters of the 532-nm and 1064-nm excitations were similar, indicating that the IR band is responsible for laser action for both excitations.

Comparison of Antibacterial Effects of 810 and 980- nanometer Diode Lasers on Enterococcus Faecalis in the Root Canal System -An in vitro study.

PubMed

Asnaashari, Mohamad; Ebad, Leila Tahmasebi; Shojaeian, Shiva

2016-10-01

Background and aim: Use of laser technology in endodontics has greatly increased in the recent years due to the introduction of new wavelengths and methods and optimal antimicrobial and smear layer removal properties of lasers. This in vitro study aimed to compare the antibacterial effects of diode lasers of 810 nm and 980 nm wavelength on Enterococcus faecalis (E. faecalis) biofilm in the root canal system. Materials and methods: Fifty single-canal human anterior teeth were cleaned, shaped, sterilized and randomly divided into four groups namely two experimental, one positive and one negative control group. The experimental and positive control groups were inoculated with E. faecalis and incubated for two weeks. The experimental group one (n=20) received 810 nm diode laser irradiation (1.5W) while the experimental group two (n=20) was subjected to 980 nm diode laser irradiation (1.5W). The E. faecalis colony forming units (CFUs) were counted in each root canal before and after laser irradiation. Results: Laser irradiation significantly decreased the bacterial colony count in both experimental groups. The reduction in microbial count was significantly greater in 810 nm laser group compared to 980 nm laser group. Conclusion: Irradiation of both 810 and 980 nm lasers significantly decreased the E. faecalis count in the root canal system; 810 nm laser was more effective in decreasing the intracanal microbial load.

Comparison of Antibacterial Effects of 810 and 980- nanometer Diode Lasers on Enterococcus Faecalis in the Root Canal System —An in vitro study

PubMed Central

Asnaashari, Mohamad; Ebad, Leila Tahmasebi

2016-01-01

Background and aim: Use of laser technology in endodontics has greatly increased in the recent years due to the introduction of new wavelengths and methods and optimal antimicrobial and smear layer removal properties of lasers. This in vitro study aimed to compare the antibacterial effects of diode lasers of 810 nm and 980 nm wavelength on Enterococcus faecalis (E. faecalis) biofilm in the root canal system. Materials and methods: Fifty single-canal human anterior teeth were cleaned, shaped, sterilized and randomly divided into four groups namely two experimental, one positive and one negative control group. The experimental and positive control groups were inoculated with E. faecalis and incubated for two weeks. The experimental group one (n=20) received 810 nm diode laser irradiation (1.5W) while the experimental group two (n=20) was subjected to 980 nm diode laser irradiation (1.5W). The E. faecalis colony forming units (CFUs) were counted in each root canal before and after laser irradiation. Results: Laser irradiation significantly decreased the bacterial colony count in both experimental groups. The reduction in microbial count was significantly greater in 810 nm laser group compared to 980 nm laser group. Conclusion: Irradiation of both 810 and 980 nm lasers significantly decreased the E. faecalis count in the root canal system; 810 nm laser was more effective in decreasing the intracanal microbial load. PMID:27853346

Isotope shifts from collinear laser spectroscopy of doubly charged yttrium isotopes

NASA Astrophysics Data System (ADS)

Vormawah, L. J.; Vilén, M.; Beerwerth, R.; Campbell, P.; Cheal, B.; Dicker, A.; Eronen, T.; Fritzsche, S.; Geldhof, S.; Jokinen, A.; Kelly, S.; Moore, I. D.; Reponen, M.; Rinta-Antila, S.; Stock, S. O.; Voss, A.

2018-04-01

Collinear laser spectroscopy has been performed on doubly charged ions of radioactive yttrium in order to study the isotope shifts of the 294.6-nm 5 s 1/2 2S →5 p 1/2 2P line. The potential of such an alkali-metal-like transition to improve the reliability of atomic-field-shift and mass-shift factor calculations, and hence the extraction of nuclear mean-square radii, is discussed. Production of yttrium ion beams for such studies is available at the IGISOL IV Accelerator Laboratory, Jyväskylä, Finland. This newly recommissioned facility is described here in relation to the on-line study of accelerator-produced short-lived isotopes using collinear laser spectroscopy and application of the technique to doubly charged ions.

Optogalvanic effect and laser-induced current oscillations in hollow-cathode lamps

NASA Astrophysics Data System (ADS)

Eldakli, Mohsan S. A.; Ivković, Saša S.; Obradović, Bratislav M.

2017-03-01

This paper presents a study of two commercial hollow-cathode lamps (HCLs) with the intention of demonstrating different phenomena in gas discharges. The optogalvanic effect in both HCLs is produced by a laser diode radiated at the wavelength that corresponds to neon transition 1s2-2p2 at 659.89 nm. The voltage-current characteristics of the lamps are explained using a classical theory of hollow-cathode discharge, while the optogalvanic signal is treated as a small perturbation of the discharge current. For certain values of voltage self-sustained current oscillations are observed in one of the HCLs. In the same HCL laser-induced optogalvanic dumped oscillations are detected. A phenomenological model that includes the effective circuit parameters of the discharge is used to explain the oscillation characteristics.

Spectral irradiance of singly and doubly ionized zinc in low-intensity laser-plasma ultraviolet light sources

NASA Astrophysics Data System (ADS)

Szilagyi, John; Parchamy, Homaira; Masnavi, Majid; Richardson, Martin

2017-01-01

The absolute spectral irradiances of laser-plasmas produced from planar zinc targets are determined over a wavelength region of 150 to 250 nm. Strong spectral radiation is generated using 60 ns full-width-at-half-maximum, 1.0 μm wavelength laser pulses with incident laser intensities as low as ˜5 × 108 W cm-2. A typical radiation conversion efficiency of ˜2%/2πsr is measured. Numerical calculations using a comprehensive radiation-hydrodynamics model reveal the strong experimental spectra to originate mainly from 3d94s4p-3d94s2, 3d94s4d-3d94s4p, and 3d94p-3d94s, 3d94d-3d94p unresolved-transition arrays in singly and doubly ionized zinc, respectively.

Structural origin and laser performance of thulium-doped germanate glasses.

PubMed

Xu, Rongrong; Xu, Lin; Hu, Lili; Zhang, Junjie

2011-12-15

The structural origin and laser performance of thulium-doped germanate glasses have been studied. The investigation includes two main sections. The first part discusses the Raman spectroscopic and thermal stability of the host glass structure. The low value of the largest phonon energy (850 cm(-1)) reduces the probability of nonradiative relaxation. The large emission cross section of the Tm(3+) : (3)F(4) level (8.69 × 10(-21) cm(2)), the high quantum efficiency of the (3)F(4) level (71%), and the low nonradiative relaxation rate of the (3)F(4) → (3)H(6) transition (0.09 ms(-1)) illustrate good optical properties of the germanate glass. In the second part, the room-temperature laser action from the thulium-doped germanate glass is demonstrated when pumped by a 790 nm laser diode. The maximum output power of 346 mW and slope efficiency of 25.6% are achieved.

YAG:Er3+, CaF2:Er3+, and Er2O3 Emission Spectra Under Laser and Laser Thermal Excitation

NASA Astrophysics Data System (ADS)

Marchenko, V. M.

2018-05-01

Experimental luminescence and selective-emission (SE) spectra of YAG:Er3+ (10 at.%) and CaF2:Er3+ (1 at.%) single crystals and Er2O3 polycrystal under laser and laser thermal excitation of the Er3+-ion multiplets are compared. Luminescence spectra under resonant excitation are determined by multiplet population relaxation with the corresponding radiative and nonradiative probabilities. The form of the SE spectra is determined by the thermal population of the multiplets and the probabilities of only radiative transitions. The SE band at 800 nm (4I9/2 → 4I15/2) is an indicator of high-temperature thermal emission of Er3+ ions. The absence of this band in luminescence spectra is explained by the short lifetime of the τ(4I9/2) level of 53 ns at T = 300 K.

Laser writing of coherent colour centres in diamond

NASA Astrophysics Data System (ADS)

Chen, Yu-Chen; Salter, Patrick S.; Knauer, Sebastian; Weng, Laiyi; Frangeskou, Angelo C.; Stephen, Colin J.; Ishmael, Shazeaa N.; Dolan, Philip R.; Johnson, Sam; Green, Ben L.; Morley, Gavin W.; Newton, Mark E.; Rarity, John G.; Booth, Martin J.; Smith, Jason M.

2017-02-01

Optically active point defects in crystals have gained widespread attention as photonic systems that could be applied in quantum information technologies. However, challenges remain in the placing of individual defects at desired locations, an essential element of device fabrication. Here we report the controlled generation of single negatively charged nitrogen-vacancy (NV-) centres in diamond using laser writing. Aberration correction in the writing optics allows precise positioning of the vacancies within the diamond crystal, and subsequent annealing produces single NV- centres with a probability of success of up to 45 ± 15%, located within about 200 nm of the desired position in the transverse plane. Selected NV- centres display stable, coherent optical transitions at cryogenic temperatures, a prerequisite for the creation of distributed quantum networks of solid-state qubits. The results illustrate the potential of laser writing as a new tool for defect engineering in quantum technologies, and extend laser processing to the single-defect domain.

Rapid and reversible photoinduced switching of a rotaxane crystal

NASA Astrophysics Data System (ADS)

Chen, Kai-Jen; Tsai, Ya-Ching; Suzaki, Yuji; Osakada, Kohtaro; Miura, Atsushi; Horie, Masaki

2016-11-01

Crystalline phase transitions caused by external stimuli have been used to detect physical changes in the solid-state properties. This study presents the mechanical switching of crystals of ferrocene-containing rotaxane controlled by focused laser light. The expansion and contraction of the crystals can be driven by turning on and off laser light at 445 nm. The irradiation-induced expansion of the crystal involves elongation along the a, b and c axes at 30 °C, whereas heating of the crystal at 105 °C causes the shortening of c axis. The expansions reversibly occur and have the advantage of a rapid relaxation (reverse) process. Single-crystal X-ray crystallography reveals the detailed structural changes of the molecules, corresponding to a change in the size of the crystals on laser irradiation. This molecular crystal behaviour induced by laser irradiation, is demonstrated for the remote control of objects, namely, microparticle transport and microswitching in an electric circuit.

Localized emission from laser-irradiated defects in 2D hexagonal boron nitride

NASA Astrophysics Data System (ADS)

Hou, Songyan; Danang Birowosuto, Muhammad; Umar, Saleem; Ange Anicet, Maurice; Yingjie Tay, Roland; Coquet, Philippe; Tay, Beng Kang; Wang, Hong; Teo, Edwin Hang Tong

2018-01-01

Hexagonal boron nitride (hBN) has emerged as a promising two-dimensional (2D) material for photonics device due to its large bandgap and flexibility in nanophotonic circuits. Here, we report bright and localized luminescent centres can be engineered in hBN monolayers and flakes using laser irradiation. The transition from hBN to cBN emerges in laser irradiated hBN large monolayers while is absent in processed hBN flakes. Remarkably, the colour centres in hBN flakes exhibit room temperature cleaner single photon emissions with g 2(0) ranging from 0.20 to 0.42, a narrower line width of 1.4 nm and higher brightness compared with monolayers. Our results pave the way to engineering deterministic defects in hBN induced by laser pulse and show great prospect for application of defects in hBN used as nano-size light source in photonics.

Three-dimensional nanomechanical mapping of amorphous and crystalline phase transitions in phase-change materials.

PubMed

Grishin, Ilja; Huey, Bryan D; Kolosov, Oleg V

2013-11-13

The nanostructure of micrometer-sized domains (bits) in phase-change materials (PCM) that undergo switching between amorphous and crystalline phases plays a key role in the performance of optical PCM-based memories. Here, we explore the dynamics of such phase transitions by mapping PCM nanostructures in three dimensions with nanoscale resolution by combining precision Ar ion beam cross-sectional polishing and nanomechanical ultrasonic force microscopy (UFM) mapping. Surface and bulk phase changes of laser written submicrometer to micrometer sized amorphous-to-crystalline (SET) and crystalline-to-amorphous (RESET) bits in chalcogenide Ge2Sb2Te5 PCM are observed with 10-20 nm lateral and 4 nm depth resolution. UFM mapping shows that the Young's moduli of crystalline SET bits exceed the moduli of amorphous areas by 11 ± 2%, with crystalline content extending from a few nanometers to 50 nm in depth depending on the energy of the switching pulses. The RESET bits written with 50 ps pulses reveal shallower depth penetration and show 30-50 nm lateral and few nanometer vertical wavelike topography that is anticorrelated with the elastic modulus distribution. Reverse switching of amorphous RESET bits results in the full recovery of subsurface nanomechanical properties accompanied with only partial topography recovery, resulting in surface corrugations attributed to quenching. This precision sectioning and nanomechanical mapping approach could be applicable to a wide range of amorphous, nanocrystalline, and glass-forming materials for 3D nanomechanical mapping of amorphous-crystalline transitions.

Compact Ozone Differential Absorption Lidar (DIAL) Transmitter Using Solid-State Dye Polymers

NASA Technical Reports Server (NTRS)

Jones, Alton L., Jr.; DeYoung, Russell J.; Elsayid-Ele, Hani

2001-01-01

A new potential DIAL laser transmitter is described that uses solid-state dye laser materials to make a simpler, more compact, lower mass laser system. Two solid-state dye laser materials were tested to evaluate their performance in a laser oscillator cavity end pumped by a pulsed Nd:YAG laser at 532 nm. The polymer host polymethyl-methacrylate was injected with a pyrromethene laser dye, PM 580, or PM 597. A narrowband laser oscillator cavity was constructed to produce visible wavelengths of 578 and 600 nm which were frequency doubled into the UV region (299 or 300 nm) by using a BBO crystal, resulting in a maximum energy of 11 mJ at a wavelength of 578 nm when pumped by the Nd:YAG laser at an energy of 100 mJ (532 nm). A maximum output energy of 378 microJ was achieved in the UV region at a wavelength of 289 nm but lasted only 2000 laser shots at a repetition rate of 10 Hz. The results are promising and show that a solid-state dye laser based ozone DIAL system is possible with improvements in the design of the laser transmitter.

High-power ultralong-wavelength Tm-doped silica fiber laser cladding-pumped with a random distributed feedback fiber laser

PubMed Central

Jin, Xiaoxi; Du, Xueyuan; Wang, Xiong; Zhou, Pu; Zhang, Hanwei; Wang, Xiaolin; Liu, Zejin

2016-01-01

We demonstrated a high-power ultralong-wavelength Tm-doped silica fiber laser operating at 2153 nm with the output power exceeding 18 W and the slope efficiency of 25.5%. A random distributed feedback fiber laser with the center wavelength of 1173 nm was employed as pump source of Tm-doped fiber laser for the first time. No amplified spontaneous emissions or parasitic oscillations were observed when the maximum output power reached, which indicates that employing 1173 nm random distributed feedback fiber laser as pump laser is a feasible and promising scheme to achieve high-power emission of long-wavelength Tm-doped fiber laser. The output power of this Tm-doped fiber laser could be further improved by optimizing the length of active fiber, reflectivity of FBGs, increasing optical efficiency of pump laser and using better temperature management. We also compared the operation of 2153 nm Tm-doped fiber lasers pumped with 793 nm laser diodes, and the maximum output powers were limited to ~2 W by strong amplified spontaneous emission and parasitic oscillation in the range of 1900–2000 nm. PMID:27416893

High-power ultralong-wavelength Tm-doped silica fiber laser cladding-pumped with a random distributed feedback fiber laser.

PubMed

Jin, Xiaoxi; Du, Xueyuan; Wang, Xiong; Zhou, Pu; Zhang, Hanwei; Wang, Xiaolin; Liu, Zejin

2016-07-15

We demonstrated a high-power ultralong-wavelength Tm-doped silica fiber laser operating at 2153 nm with the output power exceeding 18 W and the slope efficiency of 25.5%. A random distributed feedback fiber laser with the center wavelength of 1173 nm was employed as pump source of Tm-doped fiber laser for the first time. No amplified spontaneous emissions or parasitic oscillations were observed when the maximum output power reached, which indicates that employing 1173 nm random distributed feedback fiber laser as pump laser is a feasible and promising scheme to achieve high-power emission of long-wavelength Tm-doped fiber laser. The output power of this Tm-doped fiber laser could be further improved by optimizing the length of active fiber, reflectivity of FBGs, increasing optical efficiency of pump laser and using better temperature management. We also compared the operation of 2153 nm Tm-doped fiber lasers pumped with 793 nm laser diodes, and the maximum output powers were limited to ~2 W by strong amplified spontaneous emission and parasitic oscillation in the range of 1900-2000 nm.

Frequency measurement of the 2 S10-3 D12 two-photon transition in atomic 4He

NASA Astrophysics Data System (ADS)

Huang, Yi-Jan; Guan, Yu-Chan; Huang, Yao-Chin; Suen, Te-Hwei; Peng, Jin-Long; Wang, Li-Bang; Shy, Jow-Tsong

2018-03-01

We present precise frequency measurement of the 2 S10-3 D12 two-photon transition in 4He at 1009 nm. The laser source at 1009 nm is stabilized on an optical frequency comb to perform the absolute frequency measurement. The absolute frequency of 2 S10-3 D12 transition is experimentally determined to be 594 414 291.803(13) MHz with a relative uncertainty of 1.6 ×10-11 , which is more precise than previous determinations by a factor of 25. In combination with the theoretical ionization energy of the 3 D12 state, the ionization energy of the 2 S10 state is determined to be 960 332 040.823(24) MHz. In addition, the deduced 2 S10 and 2 S31 Lamb shifts are 2806.864(24) MHz and 4058.130(24) MHz, respectively, which are 1.6 times better than previous determinations, and the fine structure 3 D31-3 D12 is determined to be 101 143.889(29) MHz, improving the precedent determination by a factor of 11.

[Experimental investigation of laser plasma soft X-ray source with gas target].

PubMed

Ni, Qi-liang; Gong, Yan; Lin, Jing-quan; Chen, Bo; Cao, Jian-lin

2003-02-01

This paper describes a debris-free laser plasma soft X-ray source with a gas target, which has high operating frequency and can produce strong soft X-ray radiation. The valve of this light source is drived by a piezoelectrical ceramic whose operating frequency is up to 400 Hz. In comparison with laser plasma soft X-ray sources using metal target, the light source is debris-free. And it has higher operating frequency than gas target soft X-ray sources whose nozzle is controlled by a solenoid valve. A channel electron multiplier (CEM) operating in analog mode is used to detect the soft X-ray generated by the laser plasma source, and the CEM's output is fed to to a charge-sensitive preamplifier for further amplification purpose. Output charges from the CEM are proportional to the amplitude of the preamplifier's output voltage. Spectra of CO2, Xe and Kr at 8-14 nm wavelength which can be used for soft X-ray projection lithography are measured. The spectrum for CO2 consists of separate spectral lines originate mainly from the transitions in Li-like and Be-like ions. The Xe spectrum originating mainly from 4d-5f, 4d-4f, 4d-6p and 4d-5p transitions in multiply charged xenon ions. The spectrum for Kr consists of separate spectral lines and continuous broad spectra originating mainly from the transitions in Cu-, Ni-, Co- and Fe-like ions.

Diode-pumped continuous-wave eye-safe Nd:YAG laser at 1415 nm.

PubMed

Lee, Hee Chul; Byeon, Sung Ug; Lukashev, Alexei

2012-04-01

We describe the output performance of the 1415 nm emission in Nd:YAG in a plane-concave cavity under traditional pumping into the 4F5/2 level (808 nm) and direct in-band pumping into the 4F3/2 level (885 nm). An end-pumped Nd:YAG laser yielded maximum cw output power of 6.3 W and 4.2 W at 885 nm and 808 nm laser diode (LD) pumping, respectively. To the best of our knowledge, this is the highest output power of a LD-pumped 1415 nm laser.

Wide-area mapping of resting state hemodynamic correlations at microvascular resolution with multi-contrast optical imaging (Conference Presentation)

NASA Astrophysics Data System (ADS)

Senarathna, Janaka; Hadjiabadi, Darian; Gil, Stacy; Thakor, Nitish V.; Pathak, Arvind P.

2017-02-01

Different brain regions exhibit complex information processing even at rest. Therefore, assessing temporal correlations between regions permits task-free visualization of their `resting state connectivity'. Although functional MRI (fMRI) is widely used for mapping resting state connectivity in the human brain, it is not well suited for `microvascular scale' imaging in rodents because of its limited spatial resolution. Moreover, co-registered cerebral blood flow (CBF) and total hemoglobin (HbT) data are often unavailable in conventional fMRI experiments. Therefore, we built a customized system that combines laser speckle contrast imaging (LSCI), intrinsic optical signal (IOS) imaging and fluorescence imaging (FI) to generate multi-contrast functional connectivity maps at a spatial resolution of 10 μm. This system comprised of three illumination sources: a 632 nm HeNe laser (for LSCI), a 570 nm ± 5 nm filtered white light source (for IOS), and a 473 nm blue laser (for FI), as well as a sensitive CCD camera operating at 10 frames per second for image acquisition. The acquired data enabled visualization of changes in resting state neurophysiology at microvascular spatial scales. Moreover, concurrent mapping of CBF and HbT-based temporal correlations enabled in vivo mapping of how resting brain regions were linked in terms of their hemodynamics. Additionally, we complemented this approach by exploiting the transit times of a fluorescent tracer (Dextran-FITC) to distinguish arterial from venous perfusion. Overall, we demonstrated the feasibility of wide area mapping of resting state connectivity at microvascular resolution and created a new toolbox for interrogating neurovascular function.

Controlled feasibility trial comparing the use of 1470nm and 940nm diode laser for the treatment of hyperplastic inferior nasal turbinates

NASA Astrophysics Data System (ADS)

Sroka, Ronald; Havel, Miriam; Leunig, Andreas; Betz, Christian S.

2012-02-01

Introduction: So far various laser systems have been used for volume reduction of hyperplastic nasal turbinates. In case of endonasal application, fiber controlled diode lasers are preferred due to reasons of cost and practicability. The aim of this clinical study was to compare the coagulative tissue effects using either λ=1470nm vs. λ=940nm emitting lasers in treatment of hyperplastic inferior nasal turbinates in an intraindividual manner. Patients and methods: This prospective, randomized, double-blind, clinical feasibility trial included 20 patients suffering from hyperplastic inferior nasal turbinates. In each case, one nasal cavity was treated using 1470nm laser at 4- 5W, the other one with 940nm laser at 12W. Treatment was performed endoscopically controlled in non-contact mode. Clinical presentation and patients symptoms were documented preoperatively and on day 1, 3, 7, 14 and 21 postoperatively using rhinomanometry, standardized questionnaires including SNOT 20 GAV (German adapted version), and separate endoscopic examination respectively. Results: None of the patients showed infections, hemorrhages or other complications occurred intra- or postoperatively. The mean operation time was significantly shorter using the 1470nm diode laser as compared to the 940nm laser, thus lower energy was applied. There was a significant reduction of nasal obstruction on day 21 postoperatively compared to the preoperative condition on both sides regardless of the laser system used. Evaluation of the SNOT-Scores as assessed before and three weeks after surgery showed significant subjective improvements. Conclusion: Compared with standard application of 940nm diode laser, 1470nm diode laser application provides an equivalent tissue reduction in shorter operation time using less total energy and a comparable relief of nasal obstruction postoperatively.

Spectra of 42S1/2→32D5/2 Transitions of a Single Trapped 40Ca+ Ion

NASA Astrophysics Data System (ADS)

Gong, Shi-Jie; Zhou, Fei; Wu, Hao-Yu; Wan, Wei; Chen, Liang; Feng, Mang

2015-01-01

We investigate the spectra of the electric quadrupole 42S1/2→32D5/2 transitions in a single 40Ca+ ion confined in a home-built linear trap. We probe the transitions with an ultra-narrow bandwidth laser at 729 nm. In a weak magnetic field, the quadrupole transition splits into ten components with the maximal line strength proportional to their squared Clebsch—Gordan factors. In a magnetic field of the order of Gauss, the observed equidistant sideband reflects the Zeeman substructure modulated by the quantized oscillation due to the secular motion in the trap. The temperature of the trapped ion can be determined by the envelope of the sideband spectrum. We also demonstrate the Rabi oscillation in a carrier transition after the ion has been Doppler cooled, which can be fitted by the model with the thermal state of motion.

A High Power, Frequency Tunable Colloidal Quantum Dot (CdSe/ZnS) Laser

PubMed Central

Prasad, Saradh; Saleh AlHesseny, Hanan; AlSalhi, Mohamad S.; Devaraj, Durairaj; Masilamai, Vadivel

2017-01-01

Tunable lasers are essential for medical, engineering and basic science research studies. Most conventional solid-state lasers are capable of producing a few million laser shots, but limited to specific wavelengths, which are bulky and very expensive. Dye lasers are continuously tunable, but exhibit very poor chemical stability. As new tunable, efficient lasers are always in demand, one such laser is designed with various sized CdSe/ZnS quantum dots. They were used as a colloid in tetrahydrofuran to produce a fluorescent broadband emission from 520 nm to 630 nm. The second (532 nm) and/or third harmonic (355 nm) of the Nd:YAG laser (10 ns, 10 Hz) were used together as the pump source. In this study, different sized quantum dots were independently optically pumped to produce amplified spontaneous emission (ASE) with 4 nm to 7 nm of full width at half-maximum (FWHM), when the pump power and focusing were carefully optimized. The beam was directional with a 7 mrad divergence. Subsequently, these quantum dots were combined together, and the solution was placed in a resonator cavity to obtain a laser with a spectral width of 1 nm and tunable from 510 to 630 nm, with a conversion efficiency of about 0.1%. PMID:28336863

A High Power, Frequency Tunable Colloidal Quantum Dot (CdSe/ZnS) Laser.

PubMed

Prasad, Saradh; AlHesseny, Hanan Saleh; AlSalhi, Mohamad S; Devaraj, Durairaj; Masilamai, Vadivel

2017-01-30

Tunable lasers are essential for medical, engineering and basic science research studies. Most conventional solid-state lasers are capable of producing a few million laser shots, but limited to specific wavelengths, which are bulky and very expensive. Dye lasers are continuously tunable, but exhibit very poor chemical stability. As new tunable, efficient lasers are always in demand, one such laser is designed with various sized CdSe/ZnS quantum dots. They were used as a colloid in tetrahydrofuran to produce a fluorescent broadband emission from 520 nm to 630 nm. The second (532 nm) and/or third harmonic (355 nm) of the Nd:YAG laser (10 ns, 10 Hz) were used together as the pump source. In this study, different sized quantum dots were independently optically pumped to produce amplified spontaneous emission (ASE) with 4 nm to 7 nm of full width at half-maximum (FWHM), when the pump power and focusing were carefully optimized. The beam was directional with a 7 mrad divergence. Subsequently, these quantum dots were combined together, and the solution was placed in a resonator cavity to obtain a laser with a spectral width of 1 nm and tunable from 510 to 630 nm, with a conversion efficiency of about 0.1%.

Efficiency of soft tissue incision with a novel 445-nm semiconductor laser.

PubMed

Braun, Andreas; Kettner, Moritz; Berthold, Michael; Wenzler, Johannes-Simon; Heymann, Paul Günther Baptist; Frankenberger, Roland

2018-01-01

Using a 445-nm semiconductor laser for tissue incision, an effective cut is expected due to the special absorption properties of blue laser light in soft tissues. The aim of the present study was the histological evaluation of tissue samples after incision with a 445-nm diode laser. Forty soft tissue specimens were obtained from pork oral mucosa and mounted on a motorized linear translation stage. The handpiece of a high-frequency surgery device, a 970-nm semiconductor laser, and a 445-nm semiconductor laser were connected to the slide, allowing a constant linear movement (2 mm/s) and the same distance of the working tip to the soft tissue's surface. Four incisions were made each: (I) 970-nm laser with conditioned fiber tip, contact mode at 3-W cw; (II-III): 445-nm laser with non-conditioned fiber tip, contact mode at 2-W cw, and non-contact mode (1 mm) at 2 W; and (IV): high-frequency surgery device with straight working tip, 90° angulation, contact mode at 50 W. Histological analysis was performed after H&E staining of the embedded specimens at 35-fold magnification. The comparison of the incision depths showed a significant difference depending on the laser wavelength and the selected laser parameters. The highest incision depth was achieved with the 445-nm laser contact mode (median depth 0.61 mm, min 0.26, max 1.17, interquartile range 0.58) (p < 0.05) with the lowest amount of soft tissue denaturation (p < 0.05). The lowest incision depth was measured for the high-frequency surgical device (median depth 0.36 mm, min 0.12, max 1.12, interquartile range 0.23) (p < 0.05). Using a 445-nm semiconductor laser, a higher cutting efficiency can be expected when compared with a 970-nm diode laser and high-frequency surgery. Even the 445-nm laser application in non-contact mode shows clinically acceptable incision depths without signs of extensive soft tissue denaturation.

Comparison of 193 nm and 308 nm laser liquid printing by shadowgraphy imaging

NASA Astrophysics Data System (ADS)

Palla-Papavlu, A.; Shaw-Stewart, J.; Mattle, T.; Dinca, V.; Lippert, T.; Wokaun, A.; Dinescu, M.

2013-08-01

Over the last years laser-induced forward transfer has emerged as a versatile and powerful tool for engineering surfaces with active compounds. Soft, easily damageable materials can be transferred using a triazene polymer as a sacrificial layer which acts as a pressure generator and at the same time protects the material from direct laser irradiation. To understand and optimize the transfer process of biomolecules in liquid solution by using an intermediate triazene polymer photosensitive layer, shadowgraphy imaging is carried out. Two laser systems i.e. an ArF laser operating at 193 nm and a XeCl laser operating at 308 nm are applied for the transfer. Solutions with 50% v/v glycerol concentration are prepared and the influence of the triazene polymer sacrificial layer thickness (60 nm) on the deposits is studied. The shadowgraphy images reveal a pronounced difference between laser-induced forward transfer using 193 nm or 308 nm, i.e. very different shapes of the ejected liquid.

Ablative Fractional 10 600 nm Carbon Dioxide Laser Versus Non-ablative Fractional 1540 nm Erbium-Glass Laser in Egyptian Post-acne Scar patients.

PubMed

Elsaie, Mohamed L; Ibrahim, Shady M; Saudi, Wael

2018-01-01

Introduction: Non-ablative fractional erbium-doped glass 1540 nm and fractional ablative 10600 nm carbon dioxide lasers are regarded as effective modalities for treating acne atrophic scars. In this study, we aimed to compare the effectiveness of fractional CO 2 laser and fractional nonablative 1540 nm erbium doped glass laser in treating post acne atrophic scars in Egyptian patients. Methods: Fifty-eight patients complaining of moderate and severe acne atrophic scars were randomly divided into 2 groups of 29 patients each. Both groups were subjected to 4 treatment sessions with 3 weeks interval and were followed up for 3 months. In group A, enrolled patient sreceived C2 laser, while in group B, patients were treated with 1540 nm erbium glass fractional laser. Results: Clinical assessment revealed that the mean grades of progress and improvement were higher with fractional 10600 nm CO2 laser but with non-significant difference between both treatments ( P = 0.1). The overall patients' satisfaction with both lasers were not significantly different ( P = 0.44). Conclusion: Both fractional ablative CO2 and fractional non-ablative erbium glass lasers are good modalities for treating acne scars with a high efficacy and safety profile and good patient satisfaction. The fractional ablative laser showed higher efficacy while non-ablative laser offered less pain and shorter downtime.

Comparison of a novel high-power blue diode laser (λ=442 nm) with Ho:YAG (λ=2100 nm), Tm fiber (λ=1940 nm), and KTP (λ=532 nm) lasers for soft tissue ablation

NASA Astrophysics Data System (ADS)

Vinnichenko, Victoriya; Kovalenko, Anastasiya; Arkhipova, Valeriya; Yaroslavsky, Ilya; Altshuler, Gregory; Gapontsev, Valentin

2018-02-01

Three lasers were directly compared, including the Ho:YAG laser (λ = 2100 nm), Tm fiber laser (λ = 1940 nm) operating in 3 different modes (CW, regular pulse, and super pulse), and blue diode laser (λ = 442 nm) for vaporization and coagulation efficiency for treating blood-rich soft tissues, ex vivo, in a porcine kidney model at quasi-contact cutting in water. In addition, experimental results were compared with published data on performance of KTP laser (λ = 532 nm) at similar experimental settings (Power = 60 W and cutting speed = 2 mm/s). Tm fiber laser in pulsed mode and blue laser produced highest vaporization rates of 3.7 and 3.4 mm3/s, respectively. Tm fiber laser (in both CW and pulsed modes) also produced the largest coagulation zone among the laser sources tested. A carbonization zone was observed for Tm fiber laser in CW and pulsed modes, as well as for the blue diode laser. Tm fiber laser in super-pulse mode and Ho:YAG laser both resulted in irregular coagulation zones without carbonization. Comparison with known data for KTP laser revealed that tissue effects of the blue laser are similar to that of the KTP laser. These results suggest that the combination of the two lasers (Tm fiber and blue diode) in one system may achieve high cutting efficiency and optimal coagulation for hemostasis during surgical treatment. Ex vivo testing of the combined system revealed feasibility of this approach. The combination of the CW Tm fiber laser (120W) and the blue diode laser (60W) emitting through a combination tip were compared with CW 120 W Tm fiber laser alone and 120 W Ho:YAG laser. Vaporization rates measured 34, 28, and 6 mm3/s, and coagulation zones measured 0.6, 1.3, and 1.7 mm, respectively. A carbonization zone was only observed with CW Tm fiber laser. The vaporization rate of combined CW Tm fiber laser / blue diode laser was comparable to published data for KTP laser for equivalent total power. Thus, high-power blue diode laser, Tm fiber laser, and their combination may provide an alternative to conventional Ho:YAG and KTP lasers for applications in urology and other surgical fields.

Near-infrared lasers and self-frequency-doubling in Nd:YCOB cladding waveguides.

PubMed

Ren, Yingying; Chen, Feng; Vázquez de Aldana, Javier R

2013-05-06

A design of cladding waveguides in Nd:YCOB nonlinear crystals is demonstrated in this work. Compact Fabry-Perot oscillation cavities are employed for waveguide laser generation at 1062 nm and self-frequency-doubling at 531 nm, under optical pump at 810 nm. The waveguide laser shows slope efficiency as high as 55% at 1062 nm. The SFD green waveguide laser emits at 531 nm with a maximum power of 100 μW.

Enhancement of luminescence properties in Er3+ doped TeO2-Na2O-PbX (X=O and F) ternary glasses.

PubMed

Kumar, Kaushal; Rai, S B; Rai, D K

2007-04-01

An enhancement of luminescence properties in Er3+ doped ternary glasses is observed on the addition of PbO/PbF2. The infrared to visible upconversion emission bands are observed at 410, 525, 550 and 658 nm, due to the 2H9/2-->4I15/2, 2H11/2-->4I15/2, 4S3/2-->4I15/2, 4F9/2-->4I15/2 transitions respectively, on excitation with 797 nm laser line. A detailed study reveals that the 2H9/2-->4I15/2 transition arises due to three step upconversion process while other transitions arise due to two step absorption. On excitation with 532 nm radiation, ultraviolet and violet upconversion bands centered at 380, 404, 410 and 475 nm wavelengths are observed along with one photon luminescence bands at 525, 550, 658 and 843 nm wavelengths. These bands are found due to the 4G11/2-->4I15/2, 2P3/2-->4I13/2, 2H9/2-->4I15/2, 2P3/2-->4I11/2, 2H11/2-->4I15/2, 4S3/2-->4I15/2, 4F9/2-->4I15/2 and 4S3/2-->4I13/2 transitions, respectively. Though incorporation of PbO and PbF2 both enhances fluorescence intensities however, PbF2 content has an important influence on upconversion luminescence emission. The incorporation of PbF2 enhances the red emission (658 nm) intensity by 1.5 times and the violet emission (410 nm) intensity by 2.0 times. A concentration dependence study of fluorescence reveals the rapid increase in the red (4F9/2-->4I15/2) emission intensity relative to the green (4S3/2-->4I15/2) emission with increase in the Er3+ ion concentration. This behaviour has been explained in terms of an energy transfer by relaxation between excited ions.

Nonlinear excitation fluorescence microscopy: source considerations for biological applications

NASA Astrophysics Data System (ADS)

Wokosin, David L.

2008-02-01

Ultra-short-pulse solid-state laser sources have improved contrast within fluorescence imaging and also opened new windows of investigation in biological imaging applications. Additionally, the pulsed illumination enables harmonic scattering microscopy which yields intrinsic structure, symmetry and contrast from viable embryos, cells and tissues. Numerous human diseases are being investigated by the combination of (more) intact dynamic tissue imaging of cellular function with gene-targeted specificity and electrophysiology context. The major limitation to more widespread use of multi-photon microscopy has been the complete system cost and added complexity above and beyond commercial camera and confocal systems. The current status of all-solid-state ultrafast lasers as excitation sources will be reviewed since these lasers offer tremendous potential for affordable, reliable, "turnkey" multiphoton imaging systems. This effort highlights the single box laser systems currently commercially available, with defined suggestions for the ranges for individual laser parameters as derived from a biological and fluorophore limited perspective. The standard two-photon dose is defined by 800nm, 10mW, 200fs, and 80Mhz - at the sample plane for tissue culture cells, i.e. after the full scanning microscope system. Selected application-derived excitation wavelengths are well represented by 700nm, 780nm, ~830nm, ~960nm, 1050nm, and 1250nm. Many of the one-box lasers have fixed or very limited excitation wavelengths available, so the lasers will be lumped near 780nm, 800nm, 900nm, 1050nm, and 1250nm. The following laser parameter ranges are discussed: average power from 200mW to 2W, pulse duration from 70fs to 700fs, pulse repetition rate from 20MHz to 200MHz, with the laser output linearly polarized with an extinction ratio at least 100:1.

Optical design of f-theta lens for dual wavelength selective laser melting

NASA Astrophysics Data System (ADS)

Feng, Lianhua; Cao, Hongzhong; Zhang, Ning; Xu, Xiping; Duan, Xuanming

2016-10-01

F-theta lens is an important unit for selective laser melting (SLM) manufacture. The dual wavelength f-theta lens has not been used in SLM manufacture. Here, we present the design of the f-theta lens which satisfies SLM manufacture with coaxial 532 nm and 1030 nm 1080 nm laser beams. It is composed of three pieces of spherical lenses. The focal spots for 532 nm laser and 1030 nm 1080 nm laser are smaller than 35 μm and 70 μm, respectively. The results meet the demands of high precision SLM. The chromatic aberration could cause separation between two laser focal spots in the scanning plane, so chromatic aberration correction is very important to our design. The lateral color of the designed f-theta lens is less than 11 μm within the scan area of 150 mm x 150 mm, which meet the application requirements of dual wavelength selective laser melting.

Future directions in 980-nm pump lasers: submarine deployment to low-cost watt-class terrestrial pumps

NASA Astrophysics Data System (ADS)

Gulgazov, Vadim N.; Jackson, Gordon S.; Lascola, Kevin M.; Major, Jo S.; Parke, Ross; Richard, Tim; Rossin, Victor V.; Zhang, Kai

1999-09-01

The demands of global bandwidth and distribution are rising rapidly as Internet usage grows. This fundamentally means that more photons are flowing within optical cables. While transmitting sources launches some optical power, the majority of the optical power that is present within modern telecommunication systems originates from optical amplifiers. In addition, modern optical amplifiers offer flat optical gain over broad wavelength bands, thus making possible dense wavelength de-multiplexing (DWDM) systems. Optical amplifier performance, and by extension the performance of the laser pumps that drive them, is central to the future growth of both optical transmission and distribution systems. Erbium-doped amplifiers currently dominate optical amplifier usage. These amplifiers absorb pump light at 980 nm and/or 1480 nm, and achieve gain at wavelengths around 1550 nm. 980 nm pumps achieve better noise figures and are therefore used for the amplification of small signals. Due to the quantum defect, 1480 nm lasers deliver more signal photon per incident photon. In addition, 1480 nm lasers are less expensive than 980 nm lasers. Thus, 1480 nm pump lasers are used for amplification in situations where noise is not critical. The combination of these traits leads to the situation where many amplifiers contain 980 nm lasers to pump the input section of the Er- doped fiber with 1480 nm lasers being used to pump the latter section of Er fiber. This can be thought of as using 980 nm lasers to power an optical pre-amplifier with the power amplification function being pump with 1480 nm radiation. This paper will focus on 980 nm pump lasers and the impact that advances in 980 nm pump technology will have on optical amplification systems. Currently, 980 nm technology is rapidly advancing in two areas, power and reliability. Improving reliability is becoming increasingly important as amplifiers move towards employing more pump lasers and using these pump lasers without redundancy. Since the failure rate allowable for an amplifier is not a function of the number of pumps employed in the amplifier, the allowable failure rate of an individual pump laser is decreasing for next-generation amplifiers. This will lead to specifications for terrestrial pumps well below 1000 FIT, and may lead to the case where high power amplifiers need laser pump reliability to approach 100 FIT. In addition, 980 nm laser diodes are now being deployed in submarine systems where failure rates lower than 100 FIT are commonly specified. It is obvious that both terrestrial and submarine markets are pushing allowable failure rates for pumps for optical amplifiers to continually decrease. A second push for improvement is in the output power of 980 nm pump modules. There exist a number of motivations for increasing the output power of pump lasers. First, each additional channel in a DWDM system requires additional power. To first order, a doubling in channel count implies a doubling in pump power. Second, larger amplifiers require multiple pumps. Higher output power from pump modules allows for fewer pumps, less complicated control systems and smaller size amplifiers. The discussion of this paper will focus on how current development progress of 980 nm laser diodes addresses these issues: better reliability and higher output powers.

High power diode lasers emitting from 639 nm to 690 nm

NASA Astrophysics Data System (ADS)

Bao, L.; Grimshaw, M.; DeVito, M.; Kanskar, M.; Dong, W.; Guan, X.; Zhang, S.; Patterson, J.; Dickerson, P.; Kennedy, K.; Li, S.; Haden, J.; Martinsen, R.

2014-03-01

There is increasing market demand for high power reliable red lasers for display and cinema applications. Due to the fundamental material system limit at this wavelength range, red diode lasers have lower efficiency and are more temperature sensitive, compared to 790-980 nm diode lasers. In terms of reliability, red lasers are also more sensitive to catastrophic optical mirror damage (COMD) due to the higher photon energy. Thus developing higher power-reliable red lasers is very challenging. This paper will present nLIGHT's released red products from 639 nm to 690nm, with established high performance and long-term reliability. These single emitter diode lasers can work as stand-alone singleemitter units or efficiently integrate into our compact, passively-cooled Pearl™ fiber-coupled module architectures for higher output power and improved reliability. In order to further improve power and reliability, new chip optimizations have been focused on improving epitaxial design/growth, chip configuration/processing and optical facet passivation. Initial optimization has demonstrated promising results for 639 nm diode lasers to be reliably rated at 1.5 W and 690nm diode lasers to be reliably rated at 4.0 W. Accelerated life-test has started and further design optimization are underway.

The enhanced and broadband near-infrared emission in Pr3+/Nd3+ co-doped tellurite glass

NASA Astrophysics Data System (ADS)

Zhou, Zizhong; Zhou, Yaxun; Cheng, Pan; Zhou, Minghan; Su, Xiue; Li, Jun

2017-11-01

This paper reports an enhanced and broadband near-infrared fluorescence emission in the Pr3+/Nd3+ co-doped tellurite glass, which was prepared using melt-quenching technique. Under the excitation of 488 nm laser diode (LD), three near-infrared emission bands at around 0.9, 1.04 and 1.30 μm from 3P1,0 → 1G4, 1G4→3H4 and 1G4→3H5 radiative transitions respectively were observed in the Pr3+ single-doped glass, and the fluorescence intensities increased further with the introduction of Nd3+ ions, which is mainly attributed to the energy transfers from Nd3+ to Pr3+ emissions. Meanwhile, the spectral overlapping of Pr3+:1G4→3H4 and Nd3+:4F3/2 → 4I11/2 radiative transitions resulted in a broadband emission ranging from 1000 to 1100 nm, whose full-width at half-maximum (FWHM) reached about 66 nm. Additionally, the spectroscopic properties of Nd3+ and Pr3+ ions were analyzed using Judd-Ofelt theory and the thermal stability property of prepared glass was characterized by the differential scanning calorimeter (DSC) measurement, and larger than 134 °C for the difference ΔT(=Tx -Tg) was observed, which indicates its feasibility for later fiber drawing. The enhanced fluorescence and broadband emission indicate that Pr3+/Nd3+ co-doped tellurite glass can be applied in the near-infrared band tunable lasers and broadband optical amplifiers.

Blood oxygenation and flow measurements using a single 720-nm tunable V-cavity laser.

PubMed

Feng, Yafei; Deng, Haoyu; Chen, Xin; He, Jian-Jun

2017-08-01

We propose and demonstrate a single-laser-based sensing method for measuring both blood oxygenation and microvascular blood flow. Based on the optimal wavelength range found from theoretical analysis on differential absorption based blood oxygenation measurement, we designed and fabricated a 720-nm-band wavelength tunable V-cavity laser. Without any grating or bandgap engineering, the laser has a wavelength tuning range of 14.1 nm. By using the laser emitting at 710.3 nm and 724.4 nm to measure the oxygenation and blood flow, we experimentally demonstrate the proposed method.

Demonstration of miniaturized 20mW CW 280nm and 266nm solid-state UV laser sources

NASA Astrophysics Data System (ADS)

Landru, Nicolas; Georges, Thierry; Beaurepaire, Julien; Le Guen, Bruno; Le Bail, Guy

2015-02-01

Visible 561 nm and 532 nm laser emissions from 14-mm long DPSS monolithic cavities are frequency converted to deep UV 280 nm and 266 nm in 16-mm long monolithic external cavities. Wavelength conversion is fully insensitive to mechanical vibrations and the whole UV laser sources fit in a miniaturized housing. More than 20 mW deep UV laser emission is demonstrated with high power stability, low noise and good beam quality. Aging tests are in progress but long lifetimes are expected thanks to the cavity design. Protein detection and deep UV resonant Raman spectroscopy are applications that could benefit from these laser sources.

Twin-induced phase transition from β-Ga2O3 to α-Ga2O3 in Ga2O3 thin films

NASA Astrophysics Data System (ADS)

Choi, Byeongdae; Allabergenov, Bunyod; Lyu, Hong-Kun; Lee, Seong Eui

2018-06-01

We deposited a 300-nm-thick Ga2O3 thin film on an amorphous SiO2/Si substrate via pulsed laser deposition. X-ray diffraction patterns revealed the formation of β-Ga2O3 phase at a substrate temperature of 700 °C. X-ray photoelectron spectra indicated that the degree of oxidation increased after annealing at 700 °C. Further annealings at higher temperatures led to a transition of the β-Ga2O3 phase to the α-Ga2O3 phase; this transition was caused by the twin structure formed during the crystallinity improvement process. In addition, we discuss the mechanism of the transition from the β phase to the α phase in the β-Ga2O3 thin films.

A comparative study with a 755 nm picosecond Alexandrite laser with a diffractive lens array and a 532 nm/1064 nm Nd:YAG with a holographic optic.

PubMed

Tanghetti Md, Emil; Jennings, John

2018-01-01

This study was performed to better understand the cutaneous effects of using a fractional picosecond laser at 755 nm with a diffractive lens array and a picosecond Nd:YAG laser at 532 mn and 1064 nm with a holographic optic. We characterized the injuries created by these devices on skin clinically and histologically over 24 hours. With this information we modeled the effects of these devices on a cutaneous target. Eight patients, representing Fitzpatrick skin types I-VI, were treated on their backs with a picosecond Alexandrite laser with a diffractive lens array, as well as a picosecond Nd:YAG laser at 532 nm and 1064 nm with a holographic optic. Photographs were taken 15 minutes and 24 hours after treatments. Punch biopsies were obtained at 24 hours and examined histologically. Treatment with the picosecond Nd:YAG laser at both 532 nm and 1064 nm with the holographic optic revealed erythema and small scatted areas of petechial hemorrhage areas immediately and in many cases at 24 hours after treatment. The 755 nm picosecond Alexandrite laser with diffractive lens array produced erythema immediately after treatment, which largely dissipated 24 hours later. Histologies revealed intra-epidermal vacuoles with all three wavelengths. Fractional picosecond Nd:YAG laser at 532 nm and 1064 nm with the holographic optic showed focal areas of dermal and intra-epidermal hemorrhage with areas of vascular damage in some patients. This study demonstrates that both fractional picosecond devices produce vacuoles in the skin, which are most likely due to areas of laser induced optical breakdown (LIOB). In the patients (skin type II-IV) we observed scatter areas of hemorrhage in the skin, due to vascular damage with the 532 nm and 1064 nm, but not with 755 nm wavelengths. Lasers Surg. Med. 50:37-44, 2018. © 2017 Wiley Periodicals, Inc. © 2017 Wiley Periodicals, Inc.

Determination of elemental composition of coffee using UV-pulsed laser induced breakdown spectroscopy

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gondal, M. A., E-mail: magondal@kfupm.edu.sa; Baig, Umair; Dastageer, M. A.

A detection system based on laser induced breakdown spectroscopy (LIBS) was built using 266 nm wavelength pulsed laser from the fourth harmonic of Nd:YAG laser, 500 mm spectrograph and gated ICCD camera with built-in delay generator. The LIBS system was used to study the elemental composition in coffee available in the local market of Saudi Arabia for the detection of elements in coffee samples. The LIBS spectrum of coffee sample revealed the presence magnesium, calcium, aluminum, copper, sodium, barium, bromine, cobalt, chromium, cerium manganese and molybdenum. Atomic transition line of sodium is used to study the parametric dependence of LIBSmore » signal. The study of the dependence of LIBS signal on the laser pulse energy is proven to be linear and the dependence of LIBS signal on the time delay between the excitation and data acquisition showed a typical increase, a peak value and a decrease with the optimum excitation – acquisition delay at 400 ns.« less

Erosion rate diagnostics in ion thrusters using laser-induced fluorescence

NASA Technical Reports Server (NTRS)

Gaeta, C. J.; Matossian, J. N.; Turley, R. S.; Beattie, J. R.; Williams, J. D.; Williamson, W. S.

1993-01-01

We have used laser-induced fluorescence (LIF) to monitor the charge-exchange ion erosion of the molybdenum accelerator electrode in ion thrusters. This real-time, nonintrusive method was implemented by operating a 30cm-diam ring-cusp thruster using xenon propellant. With the thruster operating at a total power of 5 kW, laser radiation at a wavelength of 390 nm (corresponding to a ground state atomic transition of molybdenum) was directed through the extracted ion beam adjacent to the downstream surface of the molybdenum accelerator electrode. Molybdenum atoms, sputtered from this surface as a result of charge-exchange ion erosion, were excited by the laser radiation. The intensity of the laser-induced fluorescence radiation, which is proportional to the sputter rate of the molybdenum atoms, was measured and correlated with variations in thruster operating conditions such as accelerator electrode voltage, accelerator electrode current, and test facility background pressure. We also demonstrated that the LIF technique has sufficient sensitivity and spatial resolution to evaluate accelerator electrode lifetime in ground-based test facilities.

Dual-comb spectroscopy of laser-induced plasmas

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bergevin, Jenna; Wu, Tsung-Han; Yeak, Jeremy

Dual-comb spectroscopy has become a powerful spectroscopic technique in applications that rely on its broad spectral coverage combined with high frequency resolution capabilities. Experiments to date have primarily focused on detection and analysis of multiple gas species under semi-static conditions, with applications ranging from environmental monitoring of greenhouse gases to high resolution molecular spectroscopy. Here, we utilize dual-comb spectroscopy to demonstrate broadband, high-resolution, and time-resolved measurements in a laser induced plasma for the first time. As a first demonstration, we simultaneously detect trace amounts of Rb and K in solid samples with a single laser ablation shot, with transitions separatedmore » by over 6 THz (13 nm) and spectral resolution sufficient to resolve isotopic and ground state hyperfine splittings of the Rb D2 line. This new spectroscopic approach offers the broad spectral coverage found in the powerful techniques of laser-induced breakdown spectroscopy (LIBS) while providing the high-resolution and accuracy of cw laser-based spectroscopies.« less

Oxygen measurements at high pressures with vertical cavity surface-emitting lasers

NASA Astrophysics Data System (ADS)

Wang, J.; Sanders, S. T.; Jeffries, J. B.; Hanson, R. K.

Measurements of oxygen concentration at high pressures (to 10.9 bar) were made using diode-laser absorption of oxygen A-band transitions near 760 nm. The wide current-tuning frequency range (>30 cm-1) of vertical cavity surface-emitting lasers (VCSELs) was exploited to enable the first scanned-wavelength demonstration of diode-laser absorption at high pressures; this strategy is more robust than fixed-wavelength strategies, particularly in hostile environments. The wide tuning range and rapid frequency response of the current tuning were further exploited to demonstrate wavelength-modulation absorption spectroscopy in a high-pressure environment. The minimum detectable absorbance demonstrated, 1×10-4, corresponds to 800 ppm-m oxygen detectivity at room temperature and is limited by etalon noise. The rapid- and wide-frequency tunability of VCSELs should significantly expand the application domain of absorption-based sensors limited in the past by the small current-tuning frequency range (typically <2 cm-1) of conventional edge-emitting diode lasers.

Ultrafast, high repetition rate, ultraviolet, fiber-laser-based source: application towards Yb⁺ fast quantum-logic.

PubMed

Hussain, Mahmood Irtiza; Petrasiunas, Matthew Joseph; Bentley, Christopher D B; Taylor, Richard L; Carvalho, André R R; Hope, Joseph J; Streed, Erik W; Lobino, Mirko; Kielpinski, David

2016-07-25

Trapped ions are one of the most promising approaches for the realization of a universal quantum computer. Faster quantum logic gates could dramatically improve the performance of trapped-ion quantum computers, and require the development of suitable high repetition rate pulsed lasers. Here we report on a robust frequency upconverted fiber laser based source, able to deliver 2.5 ps ultraviolet (UV) pulses at a stabilized repetition rate of 300.00000 MHz with an average power of 190 mW. The laser wavelength is resonant with the strong transition in Ytterbium (Yb⁺) at 369.53 nm and its repetition rate can be scaled up using high harmonic mode locking. We show that our source can produce arbitrary pulse patterns using a programmable pulse pattern generator and fast modulating components. Finally, simulations demonstrate that our laser is capable of performing resonant, temperature-insensitive, two-qubit quantum logic gates on trapped Yb⁺ ions faster than the trap period and with fidelity above 99%.

The role of defects in laser-induced modifications of silica coatings and fused silica using picosecond pulses at 1053 nm: I Damage morphology

DOE PAGES

Laurence, T. A.; Ly, S.; Shen, N.; ...

2017-06-22

Laser-induced damage with ps pulse widths straddles the transition from intrinsic, multi-photon ionization and avalanche ionization-based ablation with fs pulses to defect-dominated, thermal-based damage with ns pulses. We investigated the morphology of damage for fused silica and silica coatings between 1 ps and 60 ps at 1053 nm. Using calibrated laser-induced damage experiments, in situ imaging, and high-resolution optical microscopy, atomic force microscopy, and scanning electron microscopy, we show that defects play an important role in laser-induced damage down to 1 ps. Three types of damage are observed: ablation craters, ultra-high density pits, and smooth, circular depressions with central pits.more » For 10 ps and longer, the smooth, circular depressions limit the damage performance of fused silica and silica coatings. The observed high-density pits and material removal down to 3 ps indicate that variations in surface properties limit the laser-induced damage onset to a greater extent than expected below 60 ps. Below 3 ps, damage craters are smoother although there is still evidence as seen by AFM of inhomogeneous laser-induced damage response very near the damage onset. These results show that modeling the damage onset only as a function of pulse width does not capture the convoluted processes leading to laser induced damage with ps pulses. It is necessary to account for the effects of defects on the processes leading to laser-induced damage. In conclusion, the effects of isolated defects or inhomogeneities are most pronounced above 3 ps but are still discernible and possibly important down to the shortest pulse width investigated here.« less

The role of defects in laser-induced modifications of silica coatings and fused silica using picosecond pulses at 1053 nm: I Damage morphology

DOE Office of Scientific and Technical Information (OSTI.GOV)

Laurence, T. A.; Ly, S.; Shen, N.

Laser-induced damage with ps pulse widths straddles the transition from intrinsic, multi-photon ionization and avalanche ionization-based ablation with fs pulses to defect-dominated, thermal-based damage with ns pulses. We investigated the morphology of damage for fused silica and silica coatings between 1 ps and 60 ps at 1053 nm. Using calibrated laser-induced damage experiments, in situ imaging, and high-resolution optical microscopy, atomic force microscopy, and scanning electron microscopy, we show that defects play an important role in laser-induced damage down to 1 ps. Three types of damage are observed: ablation craters, ultra-high density pits, and smooth, circular depressions with central pits.more » For 10 ps and longer, the smooth, circular depressions limit the damage performance of fused silica and silica coatings. The observed high-density pits and material removal down to 3 ps indicate that variations in surface properties limit the laser-induced damage onset to a greater extent than expected below 60 ps. Below 3 ps, damage craters are smoother although there is still evidence as seen by AFM of inhomogeneous laser-induced damage response very near the damage onset. These results show that modeling the damage onset only as a function of pulse width does not capture the convoluted processes leading to laser induced damage with ps pulses. It is necessary to account for the effects of defects on the processes leading to laser-induced damage. In conclusion, the effects of isolated defects or inhomogeneities are most pronounced above 3 ps but are still discernible and possibly important down to the shortest pulse width investigated here.« less

885-nm Pumped Ceramic Nd:YAG Master Oscillator Power Amplifier Laser System

NASA Technical Reports Server (NTRS)

Yu, Anthony

2012-01-01

The performance of a traditional diode pumped solid-state laser that is typically pumped with 808-nm laser diode array (LDA) and crystalline Nd:YAG was improved by using 885-nm LDAs and ceramic Nd:YAG. The advantage is lower quantum defect, which will improve the thermal loading on laser gain medium, resulting in a higher-performance laser. The use of ceramic Nd:YAG allows a higher Nd dopant level that will make up the lower absorption at the 885-nm wavelength on Nd:YAG. When compared to traditional 808-nm pump, 885-nm diodes will have 30% less thermal load (or wasted heat) and will thus see a similar percentage improvement in the overall laser efficiency. In order to provide a more efficient laser system for future flight missions that require the use of low-repetition- rate (1% Nd. To make certain that the absorption at 885 nm is on the same par as the 808-nm diode, the Nd:YAG material needs to be doped with higher concentration of Nd. Ceramic Nd:YAG is the only material that can be tailored to specific needs.

New Measurement of the 1 S -3 S Transition Frequency of Hydrogen: Contribution to the Proton Charge Radius Puzzle

NASA Astrophysics Data System (ADS)

Fleurbaey, Hélène; Galtier, Sandrine; Thomas, Simon; Bonnaud, Marie; Julien, Lucile; Biraben, François; Nez, François; Abgrall, Michel; Guéna, Jocelyne

2018-05-01

We present a new measurement of the 1 S -3 S two-photon transition frequency of hydrogen, realized with a continuous-wave excitation laser at 205 nm on a room-temperature atomic beam, with a relative uncertainty of 9 ×10-13. The proton charge radius deduced from this measurement, rp=0.877 (13 ) fm , is in very good agreement with the current CODATA-recommended value. This result contributes to the ongoing search to solve the proton charge radius puzzle, which arose from a discrepancy between the CODATA value and a more precise determination of rp from muonic hydrogen spectroscopy.

Direct observation of single layer graphene oxide reduction through spatially resolved, single sheet absorption/emission microscopy.

PubMed

Sokolov, Denis A; Morozov, Yurii V; McDonald, Matthew P; Vietmeyer, Felix; Hodak, Jose H; Kuno, Masaru

2014-06-11

Laser reduction of graphene oxide (GO) offers unique opportunities for the rapid, nonchemical production of graphene. By tuning relevant reduction parameters, the band gap and conductivity of reduced GO can be precisely controlled. In situ monitoring of single layer GO reduction is therefore essential. In this report, we show the direct observation of laser-induced, single layer GO reduction through correlated changes to its absorption and emission. Absorption/emission movies illustrate the initial stages of single layer GO reduction, its transition to reduced-GO (rGO) as well as its subsequent decomposition upon prolonged laser illumination. These studies reveal GO's photoreduction life cycle and through it native GO/rGO absorption coefficients, their intrasheet distributions as well as their spatial heterogeneities. Extracted absorption coefficients for unreduced GO are α405 nm ≈ 6.5 ± 1.1 × 10(4) cm(-1), α520 nm ≈ 2.1 ± 0.4 × 10(4) cm(-1), and α640 nm ≈ 1.1 ± 0.3 × 10(4) cm(-1) while corresponding rGO α-values are α405 nm ≈ 21.6 ± 0.6 × 10(4) cm(-1), α520 nm ≈ 16.9 ± 0.4 × 10(4) cm(-1), and α640 nm ≈ 14.5 ± 0.4 × 10(4) cm(-1). More importantly, the correlated absorption/emission imaging provides us with unprecedented insight into GO's underlying photoreduction mechanism, given our ability to spatially resolve its kinetics and to connect local rate constants to activation energies. On a broader level, the developed absorption imaging is general and can be applied toward investigating the optical properties of other two-dimensional materials, especially those that are nonemissive and are invisible to current single molecule optical techniques.

Three color laser fluorometer for studies of phytoplankton fluorescence

NASA Technical Reports Server (NTRS)

Phinney, David A.; Yentsch, C. S.; Rohrer, J.

1988-01-01

A three-color laser fluorometer has been developed for field work operations. Using two tunable dye lasers (excitation wavelengths at 440 nm and 530 nm), broadband wavelength optical filters were selected to obtain maximum fluorescence sensitivity at wavelengths greater than 675 nm (chlorophyll) and 575 + or - 15 nm (phycoerythrin). The laser fluorometer permits the measurement of phytoplankton pigments under static or flowing conditions and more closely resembles the time scales (ns) and energy levels (mW) of other laser-induced fluorescence instruments.

Compact dual-wavelength Nd:GdVO4 laser working at 1063 and 1065 nm.

PubMed

Wu, Bo; Jiang, Peipei; Yang, Dingzhong; Chen, Tao; Kong, Jian; Shen, Yonghang

2009-04-13

We report a compact diode-laser pumped Nd:GdVO(4) laser with stable dual-wavelength output at 1063 nm and 1065 nm simultaneously. Two types of resonant cavity configurations were presented to support the stable dual-wavelength operation of the laser. Using a polarization beam splitter(PBS) included T-shaped cavity, we obtained a total power output over 5 W in two orthogonal polarized beam directions with 4 W in sigma polarization (1065.5 nm) and 1 W in pi polarization (1063.1 nm). By combining a half-wave-plate with the PBS in the laser cavity, a new configuration favoring one beam direction dual-wavelength output with same polarization direction was realized. A phenomenon of further line splitting was observed in both 1065 nm and 1063 nm.

Soliton self-frequency shift controlled by a weak seed laser in tellurite photonic crystal fibers.

PubMed

Liu, Lai; Meng, Xiangwei; Yin, Feixiang; Liao, Meisong; Zhao, Dan; Qin, Guanshi; Ohishi, Yasutake; Qin, Weiping

2013-08-01

We report the first demonstration of soliton self-frequency shift (SSFS) controlled by a weak continuous-wave (CW) laser, from a tellurite photonic crystal fiber pumped by a 1560 nm femtosecond fiber laser. The control of SSFS is performed by the cross-gain modulation of the 1560 nm femtosecond laser. By varying the input power of the weak CW laser (1560 nm) from 0 to 1.17 mW, the soliton generated in the tellurite photonic crystal fiber blue shifts from 1935 to 1591 nm. The dependence of the soliton wavelength on the operation wavelength of the weak CW laser is also measured. The results show the CW laser with a wavelength tunable range of 1530-1592 nm can be used to control the SSFS generation.

Measurement of atmospheric carbon dioxide and water vapor in built-up urban areas in the Gandhinagar-Ahmedabad region in India using a portable tunable diode laser spectroscopy system.

PubMed

Roy, Anirban; Sharma, Neetesh Kumar; Chakraborty, Arup Lal; Upadhyay, Abhishek

2017-11-01

This paper reports open-path in situ measurements of atmospheric carbon dioxide at Gandhinagar (23.2156°N, 72.6369°E) and Ahmedabad (23.0225°N, 72.5714°E) in the heavily industrialized state of Gujarat in western India. Calibration-free second harmonic wavelength modulation spectroscopy (2f WMS) is used to carry out accurate and fully automated measurements. The mean values of the mole fraction of carbon dioxide at four locations were 438 ppm, 495 ppm, 550 ppm, and 740 ppm, respectively. These values are much higher than the current global average of 406.67 ppm. A 1 mW, 2004-nm vertical cavity surface-emitting laser is used to selectively interrogate the R16 transition of carbon dioxide at 2003.5 nm (4991.2585 cm -1 ). The 2f WMS signal corresponding to the gas absorption line shape is simulated using spectroscopic parameters available in the HITRAN database and relevant laser parameters that are extracted in situ from non-absorbing spectral wings of the harmonic signals. The mole fraction of carbon dioxide is extracted in real-time by a MATLAB program from least-squares fit of the simulated 2f WMS signal to the corresponding experimentally obtained signal. A 10-mW, 1392.54-nm distributed feedback laser is used at two of the locations to carry out water vapor measurements using direct absorption spectroscopy. This is the first instance of a portable tunable diode laser spectroscopy system being deployed in an urban location in India to measure atmospheric carbon dioxide and water vapor under varying traffic conditions. The measurements clearly demonstrate the need to adopt tunable diode laser spectroscopy for precise long-term monitoring of greenhouse gases in the Indian subcontinent.

Efficient blue emission of ytterbium-doped Sr5(PO4)3F under quasi-three-level intracavity pumping

NASA Astrophysics Data System (ADS)

Yang, Y.; Cao, G. H.

2012-02-01

We report an Yb:Sr5(PO4)3F (Yb:S-FAP) laser emitting at 985 nm intracavity pumped by a 912 nm diode-pumped Nd:GdVO4 laser. A 808 nm diode laser is used to pump the Nd:GdVO4 crystal emitting at 912 nm, and the Yb:S-FAP laser emitting at 985 nm intracavity pumped at 912 nm. With incident pump power of 17.5 W, intracavity second harmonic generation has been demonstrated with a power of 131 mW at 492.5 nm by using a LBO nonlinear crystal.

Synthesis, Structural Characterization and Up-Conversion Luminescence Properties of NaYF4:Er3+,Yb3+@MOFs Nanocomposites

NASA Astrophysics Data System (ADS)

Giang, Lam Thi Kieu; Marciniak, Lukasz; Huy, Tran Quang; Vu, Nguyen; Le, Ngo Thi Hong; Binh, Nguyen Thanh; Lam, Tran Dai; Minh, Le Quoc

2017-10-01

This paper describes a facile synthesis of NaYF4:Er3+,Yb3+ nanoparticles embraced in metal-organic frameworks (MOFs), known as NaYF4:Er3+, Yb3+@MOFs core/shell nanostructures, by using iron(III) carboxylate (MIL-100) and zeolitic imidazolate frameworks (ZIF-8). Morphological, structural and optical characterization of these nanostructures were investigated by field emission-scanning electron microscopy, Fourier transform infrared spectroscopy, x-ray diffraction, and up-conversion luminescence measurements. Results showed that spherical-shaped NaYF4:Er3+,Yb3+@MIL-100 nanocomposites with diameters of 150-250 nm, and rod-shaped NaYF4:Er3+,Yb3+@ZIF-8 nanocomposites with lengths of 300-550 nm, were successfully synthesized. Under a 980-nm laser excitation at room temperature, the NaYF4:Er3+,Yb3+@MOFs nanocomposites exhibited strong up-conversion luminescence with two emission bands in the green part of spectrum at 520 nm and 540 nm corresponding to the 2H11/2 → 4I15/2 and 4S3/2 → 4I15/2 transitions of Er3+ ions, respectively, and a red emission band at 655 nm corresponding to the 4F9/2 → 4I15/2 transition of Er3+ ions. The above properties of NaYF4:Er3+,Yb3+@MOFs make them promising candidates for applications in biotechnology.

Formation of surface nanolayers in chalcogenide crystals using coherent laser beams

NASA Astrophysics Data System (ADS)

Ozga, K.; Fedorchuk, A. O.; El-Naggar, A. M.; Albassam, A. A.; Kityk, V.

2018-03-01

We have shown a possibility to form laser modified surface nanolayers with thickness up to 60 nm in some ternary chalcogenide crystals (Ag3AsS3, Ag3SbS3, Tl3SbS3) The laser treatment was performed by two coherent laser beams split in a space. As the inducing lasers we have applied continuous wave (cw) Hesbnd Cd laser at wavelength 441 nm and doubled frequency cw Nd: YAG laser at 532 nm. The spectral energies of these lasers were higher with respect to the energy gaps of the studied crystals. The optical anisotropy was appeared and defected by monitoring of birefringence at probing wavelength of cw Hesbnd Ne laser at λ = 3390 nm. The changes of the laser stimulated near the surface layer morphology was monitored by TEM and AFM methods as well as by the reflected optical second harmonic generation at fundamental wavelength of microsecond CO2 laser generating at wavelength 10600 nm. This technique may open a new approach for the formation of the near the surface nanolayers in chalcogenides using external cw laser illumination.

A Compact Ti:Sapphire Laser With its Third Harmonic Generation (THG) for an Airborne Ozone Differential Absorption Lidar (DIAL) Transmitter

NASA Technical Reports Server (NTRS)

Chen, Songsheng; Storm, Mark E.; Marsh, Waverly D.; Petway, Larry B.; Edwards, William C.; Barnes, James C.

2000-01-01

A compact and high-pulse-energy Ti:Sapphire laser with its Third Harmonic Generation (THG) has been developed for an airborne ozone differential absorption lidar (DIAL) to study the distributions and concentrations of the ozone throughout the troposphere. The Ti:Sapphire laser, pumped by a frequency-doubled Nd:YAG laser and seeded by a single mode diode laser, is operated either at 867 nm or at 900 nm with a pulse repetition frequency of 20 Hz. High energy laser pulses (more than 110 mJ/pulse) at 867 nm or 900 nm with a desired beam quality have been achieved and utilized to generate its third harmonic at 289nm or 300nm, which are on-line and off-line wavelengths of an airborne ozone DIAL. After being experimentally compared with Beta-Barium Borate (beta - BaB2O4 or BBO) nonlinear crystals, two Lithium Triborate (LBO) crystals (5 x 5 x 20 cu mm) are selected for the Third Harmonic Generation (THG). In this paper, we report the Ti:Sapphire laser at 900 nm and its third harmonic at 300 nm. The desired high ultraviolet (UV) output pulse energy is more than 30 mJ at 300 nm and the energy conversion efficiency from 900 nm to 300 nm is 30%.

Quantitative Laser-Saturated Fluorescence Measurements of Nitric Oxide in a Heptane Spray Flame

NASA Technical Reports Server (NTRS)

Cooper, Clayton S.; Laurendeau, Normand M.; Lee, Chi (Technical Monitor)

1997-01-01

We report spatially resolved laser-saturated fluorescence measurements of NO concentration in a pre-heated, lean-direct injection (LDI) spray flame at atmospheric pressure. The spray is produced by a hollow-cone, pressure-atomized nozzle supplied with liquid heptane. NO is excited via the Q2(26.5) transition of the gamma(0,0) band. Detection is performed in a 2-nm region centered on the gamma(0,1) band. Because of the relatively close spectral spacing between the excitation (226 nm) and detection wavelengths (236 nm), the gamma(0,1) band of NO cannot be isolated from the spectral wings of the Mie scattering signal produced by the spray. To account for the resulting superposition of the fluorescence and scattering signals, a background subtraction method has been developed that utilizes a nearby non-resonant wavelength. Excitation scans have been performed to locate the optimum off-line wavelength. Detection scans have been performed at problematic locations in the flame to determine possible fluorescence interferences from UHCs and PAHs at both the on-line and off-line excitation wavelengths. Quantitative radial NO profiles are presented and analyzed so as to better understand the operation of lean-direct injectors for gas turbine combustors.

Electronic Transitions of Tungsten Monosulfide

NASA Astrophysics Data System (ADS)

Tsang, L. F.; Chan, Man-Chor; Zou, Wenli; Cheung, Allan S. C.

2017-06-01

Electronic transition spectrum of the tungsten monosulfide (WS) molecule in the near infrared region between 725 nm and 885 nm has been recorded using laser ablation/reaction free-jet expansion and laser induced fluorescence spectroscopy. The WS molecule was produced by reacting laser - ablated tungsten atoms with 1% CS_{2} seeded in argon. Fifteen vibrational bands with resolved rotational structure have been recorded and analyzed, which were organized into seven electronic transition systems. The ground state has been identified to be the X^{3}Σ^{-}(0^{+}) state, and the determined vibrational frequency, ΔG_{1/2} and bond length, r_{0}, are respectively 556.7 cm^{-1} and 2.0676 Å. In addition, vibrational bands belong to another transition system involving lower state with Ω = 1 component have also been analyzed. Least-squares fit of the measured line positions yielded molecular constants for the electronic states involved. The low-lying Λ-S states and Ω sub-states of WS have been calculated using state-averaged complete active space self-consistent field (SA-CASSCF) and followed by MRCISD+Q (internally contracted multi-reference configuration interaction with singles and doubles plus Davidson's cluster correction). The active space consists of 10 electrons in 9 orbitals corresponding to the W 5d6s and S 3p shells. The lower molecular orbitals from W 5s5p and S 3s are inactive but are also correlated, and relativistic effective core potential (RECPs) are adopted to replace the core orbitals with 60 (W) and 10 (S) core electrons, respectively. Spin-orbit coupling (SOC) is calculated via the state-interaction (SI) approach with RECP spin-orbit operators using SA-CASSCF wavefunctions, where the diagonal elements in the SOC matrix are replaced by the corresponding MRCISD+Q energies calculated above. Spectroscopic constants and potential energy curves of the ground and many low-lying Λ-S states and Ω sub-states of the WS molecule are obtained. The calculated spectroscopic constants of the ground and low-lying states are generally in good agreement with our experimental determination. This work represents the first experimental investigation of the electronic and molecular structure of the WS molecule.

Detection of highly toxic elements (lead and chromium) in commercially available eyeliner (kohl) using laser induced break down spectroscopy

NASA Astrophysics Data System (ADS)

Gondal, M. A.; Dastageer, M. A.; Al-Adel, F. F.; Naqvi, A. A.; Habibullah, Y. B.

2015-12-01

A sensitive laser induced breakdown spectroscopic system was developed and optimized for using it as a sensor for the detection of trace levels of lead and chromium present in the cosmetic eyeliner (kohl) of different price ranges (brands) available in the local market. Kohl is widely used in developing countries for babies as well adults for beautification as well eyes protection. The atomic transition lines at 405.7 nm and 425.4 nm were used as the marker lines for the detection of lead and chromium respectively. The detection system was optimized by finding the appropriate gate delay between the laser excitation and the data acquisition system and also by achieving optically thin plasma near the target by establishing the local thermodynamic equilibrium condition. The detection system was calibrated for these two hazardous elements and the kohl samples under investigation showed 8-15 ppm by mass of lead and 4-9 ppm by mass of Chromium, which are higher than the safe permissible levels of these elements. The limits of detection of the LIBS system for lead and chromium were found to be 1 and 2 ppm respectively.

Femtosecond laser ablation and nanoparticle formation in intermetallic NiAl

NASA Astrophysics Data System (ADS)

Jorgensen, David J.; Titus, Michael S.; Pollock, Tresa M.

2015-10-01

The ablation behavior of a stoichiometric intermetallic compound β-NiAl subjected to femtosecond laser pulsing in air has been investigated. The single-pulse ablation threshold for NiAl was determined to be 83 ± 4 mJ/cm2 and the transition to the high-fluence ablation regime occurred at 2.8 ± 0.3 J/cm2. Two sizes of nanoparticles consisting of Al, NiAl, Ni3Al and NiO were formed and ejected from the target during high-fluence ablation. Chemical analysis revealed that smaller nanoparticles (1-30 nm) tended to be rich in Al while larger nanoparticles (>100 nm) were lean in Al. Ablation in the low-fluence regime maintained this trend. Redeposited material and nanoparticles remaining on the surface after a single 3.7 J/cm2 pulse, one hundred 1.7 J/cm2 pulses, or one thousand 250 mJ/cm2 pulses were enriched in Al relative to the bulk target composition. Further, the surface of the irradiated high-fluence region was depleted in Al indicating that the fs laser ablation removal rate of the intermetallic constituents in this regime does not scale with the individual pure element ablation thresholds.

Observation of the death process of cancer cells killed through surface plasmon resonance of gold nanoring with optical coherence tomography (Conference Presentation)

NASA Astrophysics Data System (ADS)

Chen, Shih-Yang; He, Yulu; Hsieh, Cheng-Che; Hua, Wei-Hsiang; Low, Meng Chun; Tsai, Meng-Tsan; Kiang, Yean-Woei; Yang, Chih-Chung

2017-02-01

The use of a high-resolution optical coherence tomography (OCT) system with the operation wavelength around 800 nm to scan SCC4 cancer cells under different laser illumination conditions is demonstrated. The cancer cells are incubated with Au nanorings (NRIs), which are linked with photosensitizer, AlPcS, for them to be up-taken by the cells. Two Au NRI samples of different geometries for inducing localized surface plasmon (LSP) resonance around 1310 and 1064 nm are used. Four different lasers are utilized for illuminating the cells under OCT scanning, including 1310-nm continuous (cw) laser, 1064-nm cw laser, 1064-nm femtosecond (fs) laser, and 660-nm cw laser. The 1310- and 1064-nm cw lasers mainly produce the photothermal effect through the LSP resonance of Au NRIs for damaging the observed cells. Besides the photothermal effect, the 1064-nm fs laser can produce strong two-photon absorption through the assistance of the LSP resonance of Au NRI for exciting AlPcS to effectively generate singlet oxygen and damage the observed cells. The 660-nm laser can excite AlPcS through single-photon absorption for generating singlet oxygen and damaging the observed cells. With the photothermal effect, the observed cells can be killed through the process of necrosis. Through the generation of singlet oxygen, the cell membrane can be preserved and the interior substances are solidified to become a hard body of strong scattering. In this situation, the cells are killed through the apoptosis process. Illuminated by the 660-nm cw laser, a process of interior substance escape is observed through high-speed OCT scanning.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kumari, Astha, E-mail: asthaguru90@gmail.com; Rai, Vineet Kumar, E-mail: vineetkrrai@yahoo.co.in

Upconversion is an interesting optical property, generally shown by rare-earth doped materials. This unusual optical behavior shown by these rare-earths doped materials are due to their peculiar atomic configuration and electronic transitions. Here, the Tm{sup 3+}-Yb{sup 3+} codoped BaTiO{sub 3} glass with TeO{sub 2} as former has been prepared by conventional melt and quench technique and the upconversion property has been investigated with the help of near infrared (NIR) to Visible UC study. The generation of the visible UC bands around ∼ 476 nm, ∼ 653 nm, ∼ 702 nm and one NIR UC band at ∼795 nm are assignedmore » due to the {sup 1}G{sub 4}→ {sup 3}H{sub 6}, {sup 1}G{sub 4}→ {sup 3}F{sub 4}, {sup 3}F{sub 2}→ {sup 3}H{sub 6} and {sup 3}H{sub 4}→ {sup 3}H{sub 6} transitions respectively. The generations of these upconversion bands have been discussed in detail with the help of energy level diagram. The colour coordinates corresponding to the prepared material have been shown with the help of CIE chromaticity diagram. These glasses can be very appropriately used in the fabrication of solid state laser and as NIR to blue light upconverter.« less

Observed transition from Richtmyer-Meshkov jet formation through feedout oscillations to Rayleigh-Taylor instability in a laser target

NASA Astrophysics Data System (ADS)

Aglitskiy, Y.; Karasik, M.; Velikovich, A. L.; Serlin, V.; Weaver, J. L.; Kessler, T. J.; Schmitt, A. J.; Obenschain, S. P.; Nikitin, S. P.; Metzler, N.; Oh, J.

2012-10-01

Experimental study of hydrodynamic perturbation evolution triggered by a laser-driven shock wave breakout at the free rippled rear surface of a plastic target is reported. We observed a transition between two qualitatively distinct types of perturbation evolution: jet formation at low shock pressure and areal mass oscillations at high shock pressure, which correspond respectively to high and low values of effective adiabatic index. The experiments were done on the KrF Nike laser facility with laser wavelength 248 nm and a 4 ns pulse. We varied the number of beams overlapped on the plastic target to change the ablative pressure driving the shock wave through the target: 36 beams produce pressure of ˜8 Mbar, whereas a single beam irradiation reduces the pressure to ˜0.7 Mbar. With the help of side-on monochromatic x-ray imaging, planar jets manifesting the development of the Richtmyer-Meshkov-type instability in a non-accelerated target are observed at sub-megabar shock pressure. As the shock pressure exceeds 1 Mbar, instead of jet formation an oscillatory rippled expansion wave is observed, followed by the ``feedout'' of the rear-surface perturbations to the ablation front and the development of the Rayleigh-Taylor instability, which breaks up the accelerated target.

Synthesis, structural, thermal and optical properties of TeO2-Bi2O3-GeO2-Li2O glasses

NASA Astrophysics Data System (ADS)

Dimowa, Louiza; Piroeva, Iskra; Atanasova-Vladimirova, S.; Petrova, Nadia; Ganev, Valentin; Titorenkova, Rositsa; Yankov, Georgi; Petrov, Todor; Shivachev, Boris L.

2016-10-01

In this study, synthesis and characterization of novel quaternary tellurite glass system TeO2-Bi2O3-GeO2-Li2O is presented. The compositions include TeO2 and GeO2 as glass formers while different proportion of Bi2O3 and Li2O act as network modifiers. Differential thermal analysis, X-ray diffraction, scanning electron microscopy energy dispersive X-ray spectroscopy, laser ablation inductively coupled plasma mass spectrometry, UV-Vis and Raman spectroscopy are applied to study the structural, thermal and optical properties of the studied glasses. Obtained glasses possess a relatively low glass transition temperature (around 300 °C) if compared to other tellurite glasses, show good thermal transparency in the visible and near infra-red (from 2.4 to 0.4 μm) and can double the frequency of laser light from its original wavelength of 1064 nm to its second-harmonic at 532 nm (i.e. second harmonic generation).

Miniature solid-state lasers for pointing, illumination, and warning devices

NASA Astrophysics Data System (ADS)

Brown, D. C.; Singley, J. M.; Yager, E.; Kowalewski, K.; Lotito, B.; Guelzow, J.; Hildreth, J.; Kuper, J. W.

2008-04-01

In this paper we review the current status of and progress towards higher power and more wavelength diverse diode-pumped solid-state miniature lasers. Snake Creek Lasers now offers unprecedented continuous wave (CW) output power from 9.0 mm and 5.6 mm TO type packages, including the smallest green laser in the world, the MicroGreen TM laser, and the highest density green laser in the world, the MiniGreen TM laser. In addition we offer an infrared laser, the MiniIR TM, operating at 1064 nm, and have just introduced a blue Mini laser operating at 473 nm in a 9.0 mm package. Recently we demonstrated over 1 W of output power at 1064 nm from a 12 mm TO type package, and green output power from 300-500 mW from the same 12 mm package. In addition, the company is developing a number of other innovative new miniature CW solid-state lasers operating at 750 nm, 820 nm, 458 nm, and an eye-safe Q-switched laser operating at 1550 nm. We also review recently demonstrated combining volume Bragg grating (VBG) technology has been combined with automatic power control (APC) to produce high power MiniGreen TM lasers whose output is constant to +/- 10 % over a wide temperature range, without the use of a thermoelectric cooler (TEC). This technology is expected to find widespread application in military and commercial applications where wide temperature operation is particularly important. It has immediate applications in laser pointers, illuminators, and laser flashlights, and displays.

High-efficient Nd:YAG microchip laser for optical surface scanning

NASA Astrophysics Data System (ADS)

Šulc, Jan; Jelínková, Helena; Nejezchleb, Karel; Škoda, Václav

2017-12-01

A CW operating, compact, high-power, high-efficient diode pumped 1064nm laser, based on Nd:YAG active medium, was developed for optical surface scanning and mapping applications. To enhance the output beam quality, laser stability, and compactness, a microchip configuration was used. In this arrangement the resonator mirrors were deposited directly on to the laser crystal faces. The Nd-doping concentration was 1 at.% Nd/Y. The Nd:YAG crystal was 5mm long. The laser resonator without pumping radiation recuperation was investigated {the output coupler was transparent for pumping radiation. For the generated laser radiation the output coupler reflectivity was 95%@1064 nm. The diameter of the samples was 5 mm. For the laser pumping two arrangements were investigated. Firstly, a fibre coupled laser diode operating at wavelength 808nm was used in CW mode. The 400 ¹m fiber was delivering up to 14W of pump power amplitude to the microchip laser. The maximum CW output power of 7.2W @ 1064nm in close to TEM00 beam was obtained for incident pumping power 13.7W @ 808 nm. The differential efficiency in respect to the incident pump power reached 56 %. Secondly, a single-emitter, 1W laser diode operating at 808nm was used for Nd:YAG microchip pumping. The laser pumping was directly coupled into the microchip laser using free-space lens optics. Slope efficiency up to 70% was obtained in stable, high-quality, 1064nm laser beam with CW power up to 350mW. The system was successfully used for scanning of super-Gaussian laser mirrors reflectivity profile.

Green fiber lasers: An alternative to traditional DPSS green lasers for flow cytometry

PubMed Central

Telford, William G.; Babin, Sergey A.; Khorev, Serge V.; Rowe, Stephen H.

2009-01-01

Green and yellow diode-pumped solid state (DPSS) lasers (532 and 561 nm) have become common fixtures on flow cytometers, due to their efficient excitation of phycoerythrin (PE) and its tandems, and their ability to excite an expanding array of expressible red fluorescent proteins. Nevertheless, they have some disadvantages. DPSS 532 nm lasers emit very close to the fluorescein bandwidth, necessitating optical modifications to permit detection of fluorescein and GFP. DPSS 561 nm lasers likewise emit very close to the PE detection bandwidth, and also cause unwanted excitation of APC and its tandems, requiring high levels of crossbeam compensation to reduce spectral overlap into the PE tandems. In this paper, we report the development of a new generation of green fiber lasers that can be engineered to emit in the range between 532 and 561 nm. A 550 nm green fiber laser was integrated into both a BD LSR II™ cuvette and FACSVantage DiVa™ jet-in-air cell sorter. This laser wavelength avoided both the fluorescein and PE bandwidths, and provided better excitation of PE and the red fluorescent proteins DsRed and dTomato than a power-matched 532 nm source. Excitation at 550 nm also caused less incidental excitation of APC and its tandems, reducing the need for crossbeam compensation. Excitation in the 550 nm range therefore proved to be a good compromise between 532 and 561 nm sources. Fiber laser technology is therefore providing the flexibility necessary for precisely matching laser wavelengths to our flow cytometry applications. PMID:19777600

Electro-optically Q-switched dual-wavelength Nd:YLF laser emitting at 1047 nm and 1053 nm

NASA Astrophysics Data System (ADS)

Men, Shaojie; Liu, Zhaojun; Cong, Zhenhua; Li, Yongfu; Zhang, Xingyu

2015-05-01

A flash-lamp pumped electro-optically Q-switched dual-wavelength Nd:YLF laser is demonstrated. Two Nd:YLF crystals placed in two cavities are employed to generate orthogonally polarized 1047 nm and 1053 nm radiations, respectively. The two cavities are jointed together by a polarizer and share the same electro-optical Q-switch. Two narrow-band pass filters are used to block unexpected oscillations at the hold-off state of the electro-optical Q-switch. In this case, electro-optical Q-switching is able to operate successfully. With pulse synchronization realized, the maximum output energy of 66.2 mJ and 83.9 mJ are obtained for 1047 nm and 1053 nm lasers, respectively. Correspondingly, the minimum pulse width is both 17 ns for 1047 nm and 1053 nm lasers. Sum frequency generation is realized. This demonstrates the potential of this laser in difference-frequency generations to obtain terahertz wave.

Compact gain saturated plasma based X-ray lasers down to 6.9nm

NASA Astrophysics Data System (ADS)

Rocca, Jorge; Wang, Y.; Wang, S.; Rockwood, A.; Berrill, M.; Shlyaptsev, V.

2017-10-01

Plasma based soft x-ray amplifiers allow many experiments requiring bright, high energy soft x-ray laser pulses to be conducted in compact facilities. We have extended the wavelength of compact gain saturated x-ray lasers to 6.89 nm in a Ni-like Gd plasma generated by a Ti:Sa laser. Gain saturated laser operation was also obtained at 7.36 nm in Ni-like Sm. Isolectronic scaling and optimization of laser pre-pulse duration allowed us to also observe strong lasing at 6.6 nm and 6.1 nm in Ni-like Tb, and amplification at 6.4 nm and 5.89 nm in Ni-like Dy. The results were obtained by transient laser heating of solid targets with traveling wave excitation at progressively increased gracing incidence angles. We show that the optimum pump angle of incidence for collisional Ni-like lasers increases linearly with atomic number from Z =42 to Z =66, reaching 43 degrees for Ni-like Dy, in good agreement with hydrodynamic/atomic physics simulations. These results will enable single-shot nano-scale imaging and other application of sub-7 nm lasers to be performed at compact facilities. Work supported by Grant DE-FG02-4ER15592 of the Department of Energy, Office of Science, and by the National Science Foundation Grant ECCS 1509925.

Effect of a 308-nm excimer laser on atopic dermatitis-like skin lesions in NC/Nga mice.

PubMed

Oh, Chang Taek; Kwon, Tae-Rin; Seok, Joon; Choi, Eun Ja; Kim, Soon Re; Jang, Yu-Jin; Mun, Seog Kyun; Kim, Chan Woong; Lee, Sungeun; Lee, Jongmin; Kim, Myeung Nam; Choi, Sun Young; Kim, Beom Joon

2016-08-01

Atopic dermatitis (AD) is a common inflammatory skin disease that can affect all age groups. It has a relapsing course, which dramatically affects the quality of life of patients. A 308-nm excimer laser has been reported to be a safe and effective treatment for inflammatory skin diseases, although the range of potential application has not been fully explored. The purpose of this study was to evaluate the therapeutic effects of a 308-nm laser on AD-like skin lesions in NC/Nga mice. Dermatophagoides farinae-exposed NC/Nga mice with a clinical score of 12 were treated with either a 308-nm excimer laser or narrowband-UVB (NB-UVB). The effects of the 308-nm excimer laser were evaluated by dermatitis scores, skin histology, skin barrier function, and immunological parameters, including IgE and Th2-mediated cytokines. The 308-nm excimer laser significantly reduced the severity of skin lesions and decreased the total serum levels of IgE and Th2-mediated cytokines. The excimer laser also significantly reduced the inflammatory cellular infiltrate into AD-induced skin lesions. Moreover, treatment with the 308-nm excimer laser led to recovery of skin barrier function in AD-induced skin lesions. The 308-nm excimer laser can be considered a valid and safe therapeutic option for the treatment of localized AD. Lasers Surg. Med. 48:629-637, 2016. © 2016 Wiley Periodicals, Inc. © 2016 Wiley Periodicals, Inc.

Spectroscopic properties of Sm3+ doped sodium-tellurite glasses: Judd-Ofelt analysis

NASA Astrophysics Data System (ADS)

Mawlud, Saman Q.; Ameen, Mudhafar M.; Sahar, Md. Rahim; Mahraz, Zahra Ashur Said; Ahmed, Kasim F.

2017-07-01

Modifying the optical response of rare earth doped inorganic glasses for diverse optical applications is the current challenge in materials science and technology. We report the enhancement of the visible emissions of the Sm3+ ions doped sodium-tellurite (TNS) glasses. The impacts of varying Sm3+ ions concentration on the spectroscopic properties of such glass samples are evaluated. Synthesized glass samples are characterized via emission and absorption measurements. The UV-Vis-NIR absorption spectra revealed nine absorption peaks which are assigned to the transitions from the ground level (6H5/2) to 6P3/2, 4I11/2, 6F11/2, 6F9/2, 6F7/2, 6F5/2, 6F3/2, 6H15/2 and 6F1/2 excited energy levels of Sm3+ ions. Emission spectra of the prepared glass under 404 nm excitation wavelength consisted of four bands centered at 561 nm, 598 nm, 643 nm and 704 nm which are originated from 4G5/2→6HJ (J = 5/2, 7/2, 9/2 and 11/2) transitions. The experimental oscillator strengths, fexp are calculated from the area under absorption bands. Using Judd-Ofelt theory and fit process of least square, the phenomenological intensity parameters Ωλ (λ = 2, 4, 6) are obtained. In order to evaluate potential applications of Sm3+ ions in telluride glasses, the spectroscopic parameters: radiative transition probability AR, branching ratio BR, radiative life time τr and stimulated emission cross section σλ for each band are calculated. These glass compositions could be a potential candidate for lasers.

Diode-pumped Nd:GAGG-LBO laser at 531 nm

NASA Astrophysics Data System (ADS)

Zou, J.; Chu, H.; Wang, L. R.

2012-03-01

We report a green laser at 531 nm generation by intracavity frequency doubling of a continuous wave (cw) laser operation of a 1062 nm Nd:GAGG laser under in-band diode pumping at 808 nm. A LiB3O5 (LBO) crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 18.5 W, as high as 933 mW of cw output power at 531 nm is achieved. The fluctuation of the green output power was better than 3.5% in the given 4 h.

1164.4  nm and 1174.7  nm dual-wavelength Nd : GdVO4/Cr4+ : YAG/YVO4 passively Q-switched Raman microchip laser.

PubMed

Wang, Xiaojie; Wang, Xiaolei; Zheng, Zhifen; Qiao, Xihao; Dong, Jun

2018-04-20

A synchronous pulsed, dual-wavelength Raman laser at 1164.4 nm and 1174.7 nm has been demonstrated in a Nd:GdVO 4 /Cr 4+ :YAG/YVO 4 passively Q-switched Raman microchip laser (PQSRML). The 1164.4 nm and 1174.7 nm dual-wavelength first-order Stokes laser oscillation is attributed to the conversion of the 1063.2 nm and 1063.43 nm two-longitudinal-mode fundamental lasers with Raman frequency shifts of 816  cm -1 and 890  cm -1 , respectively. Stable dual-wavelength Raman laser pulses with nearly equal spectral intensities have been achieved independent of the pump power. A pulse repetition rate as high as 139.4 kHz has been achieved with T 0 =85%, and the pulse width has been shortened to 825 ps with T 0 =70%. A dual-wavelength Raman laser with sub-nanosecond pulse width and peak power of over 1 kW has been achieved in the Nd:GdVO 4 /Cr 4+ :YAG/YVO 4 PQSRML.

Large laser projection displays utilizing all-solid-state RGB lasers

NASA Astrophysics Data System (ADS)

Xu, Zuyan; Bi, Yong

2005-01-01

RGB lasers projection displays have the advantages of producing large color triangle, high color saturation and high image resolution. In this report, with more than 4W white light synthesized by red (671nm), green (532nm) and blue (473nm) lasers, a RGB laser projection display system based on diode pumped solid-state lasers is developed and the performance of brilliant and vivid DVD dynamitic pictures on 60 inch screen is demonstrated.

300-mW narrow-linewidth deep-ultraviolet light generation at 193 nm by frequency mixing between Yb-hybrid and Er-fiber lasers.

PubMed

Xuan, Hongwen; Zhao, Zhigang; Igarashi, Hironori; Ito, Shinji; Kakizaki, Kouji; Kobayashi, Yohei

2015-04-20

A narrow-linewidth, high average power deep-ultraviolet (DUV) coherent laser emitting at 193 nm is demonstrated by frequency mixing a Yb-hybrid laser with an Er-fiber laser. The Yb-hybrid laser consists of Yb-fiber lasers and an Yb:YAG amplifier. The average output power of the 193 nm laser is 310 mW at 6 kHz, which corresponds to a pulse energy of 51 μJ. To the best of our knowledge, this is the highest average power and pulse energy ever reported for a narrow-linewidth 193 nm light generated by a combination of solid-state and fiber lasers with frequency mixing. We believe this laser will be beneficial for the application of interference lithography by seeding an injection-locking ArF eximer laser.

Intraindividual comparison of 1,470 nm diode laser versus carbon dioxide laser for tonsillotomy: a prospective, randomized, double blind, controlled feasibility trial.

PubMed

Havel, Miriam; Sroka, Ronald; Englert, Elsa; Stelter, Klaus; Leunig, Andreas; Betz, Christian S

2012-09-01

The need for reduction of post-tonsillectomy hemorrhage has led to promotion of tonsillotomy techniques for tonsil tissue reduction in obstructive tonsillar hypertrophy. This trial compares ablative tissue effects using 1,470 nm diode laser and carbon dioxide laser for tonsillotomy in an intraindividual design. 21 children aged 3-13 years (mean age 6.3 years) underwent laser tonsillotomy for obstructive tonsillar hypertrophy in this double blind, prospective, randomized, clinical feasibility trial. In each of the blinded patients, tonsillotomy was performed using fiber guided 1,470 nm diode laser (contact mode, 15 W power) on the one side and carbon dioxide laser (12 W power) on the other side. An independent, blinded physician documented clinical presentation and patients' symptoms preoperatively and on Days 1, 3, 7, 14, and 21 post-operatively using standardized questionnaire including VAS for each side separately. The mean duration of operative treatment was 2.7 min using 1,470 nm laser and 4.9 min using carbon dioxide laser respectively. Intraoperative bleeding and the frequency of bipolar forceps use for intraoperative bleeding control was significantly less using 1,470 nm diode laser system. There was no difference in post-operative pain scores between the carbon dioxide laser treated and the 1,470 nm fiber guided diode laser treated side. No infections, hemorrhages or other complications occurred in the course of the 3 weeks post-operative period. A fiber-guided 1,470 nm diode laser system offers an efficient and safe method for tonsillotomy as treatment of obstructive tonsillar hypertrophy. Compared to our standard practice (carbon dioxide laser), 1,470 nm laser application provides comparable tissue ablation effects with less intraoperative bleeding and shorter operation time. Copyright © 2012 Wiley Periodicals, Inc.

Intense excitation source of blue-green laser

NASA Astrophysics Data System (ADS)

Han, Kwang S.

1986-10-01

An intense and efficient source for blue green laser useful for the space-based satellite laser applications, underwater strategic communication, and measurement of ocean bottom profile is being developed. The source in use, the hypocycloidal pinch plasma (HCP), and the dense plasma focus (DPF) can produce intense uv photons (200 to 400nm) which match the absorption spectra of both near UV and blue green dye lasers (300 to 400nm). As a result of optimization of the DPF light at 355nm, the blue green dye (LD490) laser output exceeding 4mJ was obtained at the best cavity tunning of the laser system. With the HCP pumped system a significant enhancement of the blue green laser outputs with dye LD490 and coumarin 503 has been achieved through the spectrum conversion of the pumping light by mixing a converter dye BBQ. The maximum increase of laser output with the dye mixture of LD490+BBQ and coumarin 503+BBQ was greater than 80%. In addition, the untunned near UV lasers were also obtained. The near UV laser output energy of P-terphenyl dye was 0.5mJ at lambda sub C=337nm with the bandwidth of 3n m for the pulse duration of 0.2us. Another near UV laser output energy obtained with BBQ dye was 25 mJ at lambda sub C=383nm with the bandwidth of 3nm for the pulse duration of 0.2us. Another near UV laser output energy obtained with BBQ dye was 25 mJ at lambda sub C=383nm with the bandwidth of 3nm for the pulse duration of 0.2microsec.

Diode injection - seeded, 940 nanometer (nm), titanium - sapphire laser for H2O DIAL (differential absorption lidar), measurements

NASA Technical Reports Server (NTRS)

Miller, George E.

1992-01-01

Differential absorption of laser radiation by various molecular species represents both a selective and a sensitive method of measuring specific atmospheric constituents. DIAL measurements can be carried out via two different means. Both involve using two laser pulses with slightly different wavelengths (lambda), (one lambda at a strong absorption line of the molecule of interest, the other detuned into the wing of the line), and comparing the attenuation of the pulses. One approach relies on scattering of the radiation from some conveniently located topographical target. In the other technique elastic scattering from atmospheric aerosols and particulates is used to return the radiation to the lidar receiver system. This case is referred to as the differential absorption and scattering technique, and is the technique we are interested in to measure water vapor at 940 nm. The 940 nm wavelength is extremely desirable to atmospheric scientist interested in accurate DIAL measurements of H2O in the upper and lower troposphere. Simulated measurements using approximately 940 nm and 815 nm lasers at a range of altitudes and experimental conditions are shown. By offering access to larger absorption cross-sections, injected seeded, 940 nm DIAL laser transmitters would allow for more accurate water profile measurements at altitudes from 6 to 16 km than is currently possible with 730 nm and 815 nm DIAL laser transmitters. We have demonstrated the operation of an injected seeded titanium-sapphire (TS) laser operating at approximately 940 nm with an energy of more than 90 mJ per pulse. The TS laser is pumped by a commercial, 600 mJ, 532 nm, 10 Hz Nd:YAG laser. The slope efficiency of the laser using a flat 50 percent R output coupler and a 10 m end-mirror is shown. The laser was injected seeded with a CW, AlGaAs, semiconductor diode laser which had an output of 83 mW. The CW diode seed beam was introduced into the TS laser cavity through a HR end-mirror. When the diode beam is aligned to the TS resonator, it controls the TS laser output wavelength and its spectral line width with the required resolution for DIAL applications. This work supports the need for the development of 940 nm, titanium-sapphire DIAL transmitters.

Applications of the Excimer Laser: A Review.

PubMed

Beggs, Sarah; Short, Jack; Rengifo-Pardo, Monica; Ehrlich, Alison

2015-11-01

The 308-nm excimer laser has been approved by the Food and Drug Administration for the treatment of psoriasis and vitiligo. Its ability to treat localized areas has led to many studies determining its potential in the treatment of focal diseases with inflammation or hypopigmentation. To review the different applications of the 308-nm excimer laser for treating dermatologic conditions. An extensive literature review was conducted by searching PubMed, MEDLINE, and ClinicalKey to find articles pertaining to dermatologic conditions treated with the 308-nm excimer laser. Articles published that contributed to new applications of the excimer laser were included, as well as initial studies utilizing the excimer laser. The outcomes and results were compiled for different dermatologic conditions treated with the excimer laser. The 308-nm excimer laser has a wide range of uses for focal inflammatory and hypopigmented conditions. Treatment is generally well tolerated, with few adverse reactions. Larger studies and studies evaluating the long-term effects of the 308-nm excimer laser are needed.

New 223-nm excimer laser surgical system for photorefractive keratectomy

NASA Astrophysics Data System (ADS)

Bagaev, Sergei N.; Razhev, Alexander M.; Zhupikov, Andrey A.

1999-02-01

The using of KrCl (223 nm) excimer laser in ophthalmic devices for Photorefractive Keratectomy (PRK) and phototherapeutic Keratectomy (PTK) is offered. The structure and functions of a new surgical UV ophthalmic laser systems Medilex using ArF (193 nm) or KrCl (223 nm) excimer laser for corneal surgery are presented. The systems Medilex with the new optical delivery system is used for photoablative reprofiling of the cornea to correct refraction errors (myopia, hyperopia and astigmatism) and to treat a corneal pathologies. The use of the 223 nanometer laser is proposed to have advantages over the 193 nanometer laser. The results of application of the ophthalmic excimer laser systems Medilex for treatment of myopia are presented.

Dual-wavelength waveguide lasers at 1064 and 1079 nm in Nd:YAP crystal by direct femtosecond laser writing.

PubMed

Nie, Weijie; Cheng, Chen; Jia, Yuechen; Romero, Carolina; Vázquez de Aldana, Javier R; Chen, Feng

2015-05-15

Low-loss depressed cladding waveguides have been produced in Nd:YAP laser crystal by using direct femtosecond laser writing. Under optical pump at 812 nm at room temperature, continuous-wave simultaneous dual-wavelength laser oscillations at 1064 and 1079 nm, both along TM polarization, have been realized in the waveguiding structures. It has been found that, with the variation of pump polarization, the intensity ratio of 1064 and 1079 nm emissions varies periodically, while the polarization of output dual-wavelength laser remains unchanged. The maximum output power achieved for the Nd:YAP waveguide lasers is ∼200  mW with a slope efficiency of 33.4%.

New possibilities of neodymium-doped vanadate crystals as active media for diode-pumped lasers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vlasov, V I; Garnov, S V; Zavartsev, Yu D

The spectral and lasing parameters of Nd:GdVO{sub 4}, Nd:YVO{sub 4}, and Nd:Gd{sub 0.7}Y{sub 0.3}VO{sub 4} vanadate crystals cut along the c axis are studied. Lasing is obtained for the first time in a nonselective resonator at the {sup 4}F{sub 3/2}-{sup 4}I{sub 11/2} transition at 1065.5 nm in a Nd:GdVO{sub 4} crystal. Tuning is realised in the range from 1062.3 to 1066.1 nm and two-frequency lasing is obtained. (special issue devoted to the 25th anniversary of the a.m. prokhorov general physics institute)

Surface Modified Long Period Fiber Grating Sensor for Rapid Detection of Aspergillus Niger Fungal Spores

NASA Astrophysics Data System (ADS)

Gambhir, Monika; Gupta, Shilpi; John, Priya; Mahakud, Ramakanta; Kumar, Jitendra; Prakash, Om

2018-03-01

We present development of a compact and label-free sensor based on the surface modification of copper vapor laser fabricated long period fiber gratings for detection of airborne Aspergillus niger (A. niger) fungal spores. Surface of sensors were functionalized with monoclonal glucose oxidases IgG1 for target-specific covalent binding. In process of functionalization and binding of 103 cfu/ml of pathogenic A. niger fungal spores, notable shorter wave transition in resonance wavelength from 1562.93 nm to 1555.97 nm, and significant reduction in peak loss from 61.72 dB to 57.48 dB were recorded. The implementation was cost effective and yielded instantaneous results.

Lasing characteristics of gas mixtures involving UFG: Application to nuclear pumping of lasers

NASA Technical Reports Server (NTRS)

Verdeyen, J. T.; Eden, J. G.

1980-01-01

Intense blue-green fluorescence from a structured band centered at lambda approximately 484 nm was observed from Ar, CF3I and NF3 gas mixtures excited by an electron beam. This emission was tentatively assigned to the E yields A transition of the iodine monofluoride (IF) molecule. The fluorescence efficiency of the IF(E yields A) band and the IF (E) state radiative lifetime were estimated to be approximately 6% and 15 ns, respectively. The emission band structure, the short IF(E) radiative lifetime and the Franck-Condon shift between the E and A states suggest that IF is an attractive candidate for a blue-green laser.

Diode laser based resonance ionization mass spectrometric measurement of strontium-90

NASA Astrophysics Data System (ADS)

Bushaw, B. A.; Cannon, B. D.

1997-10-01

A diode laser based scheme for the isotopically selective excitation and ionization of strontium is presented. The double-resonance excitation 5s 21S 0→5s5p 3P 1→5s6s 3S 1 is followed by photoionization at 488 nm. The isotope shifts and hyperfine structure in the resonance transitions have been accurately measured for the stable isotopes and 90Sr, with the measurement of the 90Sr shifts using sub-pg samples. Analytical tests, using graphite crucible atomization, demonstrated 90Sr detection limits of 0.8 fg and overall (optical+mass spectrometer) isotopic selectivity of >10 10 against stable strontium.

Selective emission and luminescence of Er{sub 2}O{sub 3} under intense laser excitation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Marchenko, V M; Studenikin, M I; Iskhakova, L D

2013-09-30

The microstructure of Er{sub 2}O{sub 3} polycrystals synthesised by laser heating is studied. The synthesis of erbium silicate (Er{sub 2}SiO{sub 5}) layers was observed upon interaction of Er{sub 2}O{sub 3} and SiO{sub 2} melts. The dependences of the selective emission (SE) and luminescence spectra of Er{sub 2}O{sub 3} polycrystals in the range 200 – 1700 nm on the intensity of laser-thermal (at the wavelength λ = 10.6 μm) and resonant laser (λ ≈ 975 nm) excitation are investigated. The emission of heated Er{sub 2}O{sub 3} polycrystals arises as a result of multiphonon relaxation of absorbed energy and is a superpositionmore » of the SE at the electronic-vibrational transitions of Er{sup 3+} ions and the thermal radiation of the crystal lattice. The shape of the SE spectra of Er{sub 2}O{sub 3} polycrystals in the range 400 – 1700 nm almost does not change upon laser-thermal heating from 300 to 1500 K and subsequent cooling and corresponds to the absorption spectra of Er{sup 3+} ions. With increasing temperature, the thermal radiation intensity increases faster than the SE intensity, and the shape of the Er{sub 2}O{sub 3} spectrum becomes closer to the calculated spectrum of a blackbody. The anti-Stokes luminescence spectra of Er{sup 3+} ions formed under intense laser excitation of the {sup 4}I{sub 11/2} level are explained by additional SE caused by heating of the crystal matrix due to the Stokes losses. A difference between the SE and luminescence spectra is observed at low intensities of resonant laser excitation and low temperatures, when only the Stokes luminescence occurs. The temperature dependences of the SE and luminescence spectra of Er{sub 2}O{sub 3} upon laser excitation testify to the fundamental role played by the interaction of the electronic f-shell of Er{sup 3+} ions with crystal lattice vibrations in the processes of multiphonon radiative and nonradiative relaxation. The laser-thermal synthesis is promising for inprocess variation of the chemical composition of rare-earth samples. (interaction of laser radiation with matter)« less

Experimental observation of breathing solitons and a third harmonic in a tapered photonic crystal fiber

NASA Astrophysics Data System (ADS)

Wang, F.; Yao, C. F.; Li, C. Z.; Jia, Z. X.; Li, Q.; Wu, C. F.; Ohishi, Y.; Qin, W. P.; Qin, G. S.

2018-02-01

We report the experimental observation of breathing solitons and a third harmonic in a tapered fluorotellurite photonic crystal fiber (PCF) pumped by a 1560 nm femtosecond fiber laser. The PCF has a core diameter that varies continuously along its length, resulting in a zero-dispersion wavelength that moves from 1325 nm to 906 nm over the transition region. By finely controlling the dispersion map of the tapered PCF and increasing the order of the optical solitons, their breathing behavior is observed in the frequency domain and the number of breaths goes up to 9. Furthermore, the breathing behavior of the optical soliton is transferred to the third harmonic through inter-modal phase-matched processes in the tapered PCF, and the third harmonic also breathes with an increase in the pump power.