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Sample records for on-line laser ion

  1. Resonance ionization laser ion sources for on-line isotope separators (invited).

    PubMed

    Marsh, B A

    2014-02-01

    A Resonance Ionization Laser Ion Source (RILIS) is today considered an essential component of the majority of Isotope Separator On Line (ISOL) facilities; there are seven laser ion sources currently operational at ISOL facilities worldwide and several more are under development. The ionization mechanism is a highly element selective multi-step resonance photo-absorption process that requires a specifically tailored laser configuration for each chemical element. For some isotopes, isomer selective ionization may even be achieved by exploiting the differences in hyperfine structures of an atomic transition for different nuclear spin states. For many radioactive ion beam experiments, laser resonance ionization is the only means of achieving an acceptable level of beam purity without compromising isotope yield. Furthermore, by performing element selection at the location of the ion source, the propagation of unwanted radioactivity downstream of the target assembly is reduced. Whilst advances in laser technology have improved the performance and reliability of laser ion sources and broadened the range of suitable commercially available laser systems, many recent developments have focused rather on the laser/atom interaction region in the quest for increased selectivity and/or improved spectral resolution. Much of the progress in this area has been achieved by decoupling the laser ionization from competing ionization processes through the use of a laser/atom interaction region that is physically separated from the target chamber. A new application of gas catcher laser ion source technology promises to expand the capabilities of projectile fragmentation facilities through the conversion of otherwise discarded reaction fragments into high-purity low-energy ion beams. A summary of recent RILIS developments and the current status of laser ion sources worldwide is presented. PMID:24593628

  2. Resonance ionization laser ion sources for on-line isotope separators (invited)

    SciTech Connect

    Marsh, B. A.

    2014-02-15

    A Resonance Ionization Laser Ion Source (RILIS) is today considered an essential component of the majority of Isotope Separator On Line (ISOL) facilities; there are seven laser ion sources currently operational at ISOL facilities worldwide and several more are under development. The ionization mechanism is a highly element selective multi-step resonance photo-absorption process that requires a specifically tailored laser configuration for each chemical element. For some isotopes, isomer selective ionization may even be achieved by exploiting the differences in hyperfine structures of an atomic transition for different nuclear spin states. For many radioactive ion beam experiments, laser resonance ionization is the only means of achieving an acceptable level of beam purity without compromising isotope yield. Furthermore, by performing element selection at the location of the ion source, the propagation of unwanted radioactivity downstream of the target assembly is reduced. Whilst advances in laser technology have improved the performance and reliability of laser ion sources and broadened the range of suitable commercially available laser systems, many recent developments have focused rather on the laser/atom interaction region in the quest for increased selectivity and/or improved spectral resolution. Much of the progress in this area has been achieved by decoupling the laser ionization from competing ionization processes through the use of a laser/atom interaction region that is physically separated from the target chamber. A new application of gas catcher laser ion source technology promises to expand the capabilities of projectile fragmentation facilities through the conversion of otherwise discarded reaction fragments into high-purity low-energy ion beams. A summary of recent RILIS developments and the current status of laser ion sources worldwide is presented.

  3. Resonance ionization laser ion sources for on-line isotope separators (invited).

    PubMed

    Marsh, B A

    2014-02-01

    A Resonance Ionization Laser Ion Source (RILIS) is today considered an essential component of the majority of Isotope Separator On Line (ISOL) facilities; there are seven laser ion sources currently operational at ISOL facilities worldwide and several more are under development. The ionization mechanism is a highly element selective multi-step resonance photo-absorption process that requires a specifically tailored laser configuration for each chemical element. For some isotopes, isomer selective ionization may even be achieved by exploiting the differences in hyperfine structures of an atomic transition for different nuclear spin states. For many radioactive ion beam experiments, laser resonance ionization is the only means of achieving an acceptable level of beam purity without compromising isotope yield. Furthermore, by performing element selection at the location of the ion source, the propagation of unwanted radioactivity downstream of the target assembly is reduced. Whilst advances in laser technology have improved the performance and reliability of laser ion sources and broadened the range of suitable commercially available laser systems, many recent developments have focused rather on the laser/atom interaction region in the quest for increased selectivity and/or improved spectral resolution. Much of the progress in this area has been achieved by decoupling the laser ionization from competing ionization processes through the use of a laser/atom interaction region that is physically separated from the target chamber. A new application of gas catcher laser ion source technology promises to expand the capabilities of projectile fragmentation facilities through the conversion of otherwise discarded reaction fragments into high-purity low-energy ion beams. A summary of recent RILIS developments and the current status of laser ion sources worldwide is presented.

  4. Upgrade of the resonance ionization laser ion source at ISOLDE on-line isotope separation facility: New lasers and new ion beamsa)

    NASA Astrophysics Data System (ADS)

    Fedosseev, V. N.; Berg, L.-E.; Fedorov, D. V.; Fink, D.; Launila, O. J.; Losito, R.; Marsh, B. A.; Rossel, R. E.; Rothe, S.; Seliverstov, M. D.; Sjödin, A. M.; Wendt, K. D. A.

    2012-02-01

    The resonance ionization laser ion source (RILIS) produces beams for the majority of experiments at the ISOLDE on-line isotope separator. A substantial improvement in RILIS performance has been achieved through a series of upgrade steps: replacement of the copper vapor lasers by a Nd:YAG laser; replacement of the old homemade dye lasers by new commercial dye lasers; installation of a complementary Ti:Sapphire laser system. The combined dye and Ti:Sapphire laser system with harmonics is capable of generating beams at any wavelength in the range of 210-950 nm. In total, isotopes of 31 different elements have been selectively laser-ionized and separated at ISOLDE, including recently developed beams of samarium, praseodymium, polonium, and astatine.

  5. Upgrade of the resonance ionization laser ion source at ISOLDE on-line isotope separation facility: new lasers and new ion beams.

    PubMed

    Fedosseev, V N; Berg, L-E; Fedorov, D V; Fink, D; Launila, O J; Losito, R; Marsh, B A; Rossel, R E; Rothe, S; Seliverstov, M D; Sjödin, A M; Wendt, K D A

    2012-02-01

    The resonance ionization laser ion source (RILIS) produces beams for the majority of experiments at the ISOLDE on-line isotope separator. A substantial improvement in RILIS performance has been achieved through a series of upgrade steps: replacement of the copper vapor lasers by a Nd:YAG laser; replacement of the old homemade dye lasers by new commercial dye lasers; installation of a complementary Ti:Sapphire laser system. The combined dye and Ti:Sapphire laser system with harmonics is capable of generating beams at any wavelength in the range of 210-950 nm. In total, isotopes of 31 different elements have been selectively laser-ionized and separated at ISOLDE, including recently developed beams of samarium, praseodymium, polonium, and astatine. PMID:22380244

  6. On-Line Commissioning of the HRIBF Resonant Ionization Laser Ion Source

    SciTech Connect

    Liu, Yuan; Jost, Carola U; Mendez, II, Anthony J; Stracener, Daniel W; Williams, Cecil L; Madurga, M; Miernik, Krzysztof A; Miller, D.; Padgett, S; Paulauskas, Stanley V; Gross, Carl J; Grzywacz, Robert Kazimierz; Rykaczewski, Krzysztof Piotr; Wolinska-Cichocka, Marzena

    2013-01-01

    A highly-selective resonant ionization laser ion source has been successfully commissioned at the Holifield Radioactive Ion Beam Facility, Oak Ridge National Laboratory, for the production of pure beams of short-lived nuclei for spectroscopic studies. The laser ion source provided beams of neutron-rich Ga isotopes to the Low-energy Radioactive Ion Beam Spectroscopy Station for beta decay measurements. The radioactive Ga isotopes were produced by 50-MeV proton induced fission of 238U and ionized by laser radiation using a two-step resonant ionization scheme. Isobarically pure 83Ga, 85Ga, and 86Ga beams were delivered to the experiment at approximate rates of 12000 ions/s, 100 ions/s, and 3 ions/s, respectively.

  7. First application of the Laser Ion Source and Trap (LIST) for on-line experiments at ISOLDE

    NASA Astrophysics Data System (ADS)

    Fink, D. A.; Richter, S. D.; Bastin, B.; Blaum, K.; Catherall, R.; Cocolios, T. E.; Fedorov, D. V.; Fedosseev, V. N.; Flanagan, K. T.; Ghys, L.; Gottberg, A.; Imai, N.; Kron, T.; Lecesne, N.; Lynch, K. M.; Marsh, B. A.; Mendonca, T. M.; Pauwels, D.; Rapisarda, E.; Ramos, J. P.; Rossel, R. E.; Rothe, S.; Seliverstov, M. D.; Sjödin, M.; Stora, T.; Van Beveren, C.; Wendt, K. D. A.

    2013-12-01

    The Laser Ion Source and Trap (LIST) provides a new mode of operation for the resonance ionization laser ion source (RILIS) at ISOLDE/CERN, reducing the amount of surface-ionized isobaric contaminants by up to four orders of magnitude. After the first successful on-line test at ISOLDE in 2011 the LIST was further improved in terms of efficiency, selectivity, and reliability through several off-line tests at Mainz University and at ISOLDE. In September 2012, the first on-line physics experiments to use the LIST took place at ISOLDE. The measurements of the improved LIST indicate more than a twofold increase in efficiency compared to the LIST of the 2011 run. The suppression of surface-ionized francium contaminants has enabled the first in-source laser spectroscopy of 217Po and 219Po.

  8. On-line experimental results of an argon gas cell-based laser ion source (KEK Isotope Separation System)

    NASA Astrophysics Data System (ADS)

    Hirayama, Y.; Watanabe, Y. X.; Imai, N.; Ishiyama, H.; Jeong, S. C.; Jung, H. S.; Miyatake, H.; Oyaizu, M.; Kimura, S.; Mukai, M.; Kim, Y. H.; Sonoda, T.; Wada, M.; Huyse, M.; Kudryavtsev, Yu.; Van Duppen, P.

    2016-06-01

    KEK Isotope Separation System (KISS) has been developed at RIKEN to produce neutron rich isotopes with N = 126 to study the β -decay properties for application to astrophysics. The KISS is an element-selective mass-separation system which consists of an argon gas cell-based on laser ion source for atomic number selection and an ISOL mass-separation system. The argon gas cell of KISS is a key component to stop and collect the unstable nuclei produced in a multi-nucleon transfer reaction, where the isotopes of interest will be selectively ionized using laser resonance ionization. We have performed off- and on-line experiments to study the basic properties of the gas cell as well as of the KISS. We successfully extracted the laser-ionized stable 56Fe (direct implantation of a 56Fe beam into the gas cell) atoms and 198Pt (emitted from the 198Pt target by elastic scattering with a 136Xe beam) atoms from the KISS during the commissioning on-line experiments. We furthermore extracted laser-ionized unstable 199Pt atoms and confirmed that the measured half-life was in good agreement with the reported value.

  9. Controllable Laser Ion Acceleration

    NASA Astrophysics Data System (ADS)

    Kawata, S.; Kamiyama, D.; Ohtake, Y.; Takano, M.; Barada, D.; Kong, Q.; Wang, P. X.; Gu, Y. J.; Wang, W. M.; Limpouch, J.; Andreev, A.; Bulanov, S. V.; Sheng, Z. M.; Klimo, O.; Psikal, J.; Ma, Y. Y.; Li, X. F.; Yu, Q. S.

    2016-02-01

    In this paper a future laser ion accelerator is discussed to make the laser-based ion accelerator compact and controllable. Especially a collimation device is focused in this paper. The future laser ion accelerator should have an ion source, ion collimators, ion beam bunchers, and ion post acceleration devices [Laser Therapy 22, 103(2013)]: the ion particle energy and the ion energy spectrum are controlled to meet requirements for a future compact laser ion accelerator for ion cancer therapy or for other purposes. The energy efficiency from the laser to ions is improved by using a solid target with a fine sub-wavelength structure or a near-critical density gas plasma. The ion beam collimation is performed by holes behind the solid target or a multi-layered solid target. The control of the ion energy spectrum and the ion particle energy, and the ion beam bunching would be successfully realized by a multistage laser-target interaction.

  10. Development of on-line laser power monitoring system

    NASA Astrophysics Data System (ADS)

    Ding, Chien-Fang; Lee, Meng-Shiou; Li, Kuan-Ming

    2016-03-01

    Since the laser was invented, laser has been applied in many fields such as material processing, communication, measurement, biomedical engineering, defense industries and etc. Laser power is an important parameter in laser material processing, i.e. laser cutting, and laser drilling. However, the laser power is easily affected by the environment temperature, we tend to monitor the laser power status, ensuring there is an effective material processing. Besides, the response time of current laser power meters is too long, they cannot measure laser power accurately in a short time. To be more precisely, we can know the status of laser power and help us to achieve an effective material processing at the same time. To monitor the laser power, this study utilize a CMOS (Complementary metal-oxide-semiconductor) camera to develop an on-line laser power monitoring system. The CMOS camera captures images of incident laser beam after it is split and attenuated by beam splitter and neutral density filter. By comparing the average brightness of the beam spots and measurement results from laser power meter, laser power can be estimated. Under continuous measuring mode, the average measuring error is about 3%, and the response time is at least 3.6 second shorter than thermopile power meters; under trigger measuring mode which enables the CMOS camera to synchronize with intermittent laser output, the average measuring error is less than 3%, and the shortest response time is 20 millisecond.

  11. On-line composition with laser-based techniques

    SciTech Connect

    Finch, F.T.; Hartford, A. Jr.

    1982-01-01

    Current methods for determining the composition of coal gasification streams generally involve sampling, some treatment, and inherent delay times prior to analysis. Optical instrumentation, on the other hand, provides the potential for on-line, rapid-response monitoring of gasifier streams. Among the optical technques that appear quite promising for this application are coherent anti-Stokes Raman scattering (CARS), laser-induced breakdown spectroscopy (LIBS), Fourier transform infrared spectroscopy (FTIR), laser-induced fluorescence (LIF), and synchronous detection of laser-induced fluorescence (SDLIF).

  12. Versatile Ion-polarized Techniques On-line (VITO) experiment at ISOLDE-CERN

    NASA Astrophysics Data System (ADS)

    Stachura, M.; Gottberg, A.; Johnston, K.; Bissell, M. L.; Garcia Ruiz, R. F.; Martins Correia, J.; Granadeiro Costa, A. R.; Dehn, M.; Deicher, M.; Fenta, A.; Hemmingsen, L.; Mølholt, T. E.; Munch, M.; Neyens, G.; Pallada, S.; Silva, M. R.; Zakoucky, D.

    2016-06-01

    The VITO (Versatile Ion-polarized Techniques Online) project is a new experimental setup at the ISOLDE facility at CERN. VITO is a dedicated beam line for producing laser-induced spin-polarized beams of both, atoms and ions, and it has been commissioned in response to the continuously growing demand for the use of spin-polarized beams. The new VITO beam line is a modification of the formerly existing ultra-high vacuum beam line, connecting ASPIC (Apparatus for Surface Physics and Interfaces at CERN), and it has been under construction since the beginning of 2014. Once fully commissioned, VITO will open up numerous possibilities for carrying out multidisciplinary experiments in the areas of nuclear and solid state physics, fundamental interaction physics and biophysics. In its final stage the VITO beam line will provide three fully independent experimental stations: UHV chamber for material science applications, a β-asymmetry station where highly-polarized ions will be available, and a central open-end station suitable for travelling experiments. The VITO beam line will operate in two different modes providing either beams of spin-polarized atoms or ions, or non-polarized ion beams to all three end stations operating from 10-10 mbar to 50 mbar. Recent experimental campaigns with stable and radioactive beams have allowed for testing VITO's constituent parts and have demonstrated 96% of ion beam transmission to the collection chamber installed on the central station. The first experimental results obtained with on-line Perturbed Angular Correlation (PAC) spectroscopy using 68mCu ion-beams will be briefly discussed.

  13. An ion guide laser ion source for isobar-suppressed rare isotope beams

    SciTech Connect

    Raeder, Sebastian Ames, Friedhelm; Bishop, Daryl; Bricault, Pierre; Kunz, Peter; Mjøs, Anders; Heggen, Henning; Lassen, Jens Teigelhöfer, Andrea

    2014-03-15

    Modern experiments at isotope separator on-line (ISOL) facilities like ISAC at TRIUMF often depend critically on the purity of the delivered rare isotope beams. Therefore, highly selective ion sources are essential. This article presents the development and successful on-line operation of an ion guide laser ion source (IG-LIS) for the production of ion beams free of isobaric contamination. Thermionic ions from the hot ISOL target are suppressed by an electrostatic potential barrier, while neutral radio nuclides effusing out are resonantly ionized by laser radiation within a quadrupole ion guide behind this barrier. The IG-LIS was developed through detailed thermal and ion optics simulation studies and off-line tests with stable isotopes. In a first on-line run with a SiC target a suppression of surface-ionized Na contaminants in the ion beam of up to six orders of magnitude was demonstrated.

  14. On-Line Wavelength Calibration of Pulsed Laser for CO2 Differential Absorption LIDAR

    NASA Astrophysics Data System (ADS)

    Xiang, Chengzhi; Ma, Xin; Han, Ge; Liang, Ailin; Gong, Wei

    2016-06-01

    Differential absorption lidar (DIAL) remote sensing is a promising technology for atmospheric CO2 detection. However, stringent wavelength accuracy and stability are required in DIAL system. Accurate on-line wavelength calibration is a crucial procedure for retrieving atmospheric CO2 concentration using the DIAL, particularly when pulsed lasers are adopted in the system. Large fluctuations in the intensities of a pulsed laser pose a great challenge for accurate on-line wavelength calibration. In this paper, a wavelength calibration strategy based on multi-wavelength scanning (MWS) was proposed for accurate on-line wavelength calibration of a pulsed laser for CO2 detection. The MWS conducted segmented sampling across the CO2 absorption line with appropriate number of points and range of widths by using a tunable laser. Complete absorption line of CO2 can be obtained through a curve fitting. Then, the on-line wavelength can be easily found at the peak of the absorption line. Furthermore, another algorithm called the energy matching was introduced in the MWS to eliminate the backlash error of tunable lasers during the process of on-line wavelength calibration. Finally, a series of tests was conducted to elevate the calibration precision of MWS. Analysis of tests demonstrated that the MWS proposed in this paper could calibrate the on-line wavelength of pulsed laser accurately and steadily.

  15. Progress of resonant ionization laser ion source development at GANIL

    SciTech Connect

    Henares, J. L. Huguet, Y.; Lecesne, N.; Leroy, R.; Osmond, B.; Sjödin, A. M.; Kron, T.; Schneider, F.; Wendt, K.

    2014-02-15

    SPIRAL2 (Système de Production d’Ions Radioactifs Accélérés en Ligne) is a research facility under construction at GANIL (Grand Accélérateur National d’Ions Lourds) for the production of radioactive ion beams by isotope separation on-line methods and low-energy in-flight techniques. A resonant ionization laser ion source will be one of the main techniques to produce the radioactive ion beams. GISELE (GANIL Ion Source using Electron Laser Excitation) is a test bench developed to study a fully operational laser ion source available for Day 1 operations at SPIRAL2 Phase 2. The aim of this project is to find the best technical solution which combines high selectivity and ionization efficiency with small ion beam emittance and stable long term operation. Latest results about the new ion source geometry will be presented.

  16. A resonant ionization laser ion source at ORNL

    NASA Astrophysics Data System (ADS)

    Liu, Y.; Stracener, D. W.

    2016-06-01

    Multi-step resonance laser ionization has become an essential tool for the production of isobarically pure radioactive ion beams at the isotope separator on-line (ISOL) facilities around the world. A resonant ionization laser ion source (RILIS) has been developed for the former Holifield Radioactive Ion Beam Facility (HRIBF) of Oak Ridge National Laboratory. The RILIS employs a hot-cavity ion source and a laser system featuring three grating-tuned and individually pumped Ti:Sapphire lasers, especially designed for stable and simple operation. The RILIS has been installed at the second ISOL production platform of former HRIBF and has successfully provided beams of exotic neutron-rich Ga isotopes for beta decay studies. This paper reports the features, advantages, limitations, and on-line and off-line performance of the RILIS.

  17. Applications of Ion Laser Systems

    NASA Astrophysics Data System (ADS)

    Fletcher, Peter W.

    1987-04-01

    This paper provides an introduction to the more common applications of ion laser systems. Applications discussed include photocoagulation, flow cytometry, laser disk mastering, laser doppler velocimetry, Raman spectroscopy, holography, laser light shows, large screen projection, fingerprint detection, and applications in printing such as color separation and scanning. All these applications are currently in widespread use. At the end of the paper a short review is provided of developing applications such as cardiovascular surgery and semiconductor processing.

  18. Controllable laser ion beam generation

    NASA Astrophysics Data System (ADS)

    Kamiyama, D.; Takano, M.; Nagashima, T.; Barada, D.; Gu, Y. J.; Li, X. F.; Kong, Q.; Wang, P. X.; Kawata, S.

    2016-05-01

    In intense-laser plasma interaction, several issues still remain to be solved for a future laser particle acceleration. In this paper we focus on a bunching of ion beam, which is preaccelerated by a strong electric field generated in a laser plasma interaction. In this study, a nearcritical-density plasma target is illuminated by an intense short laser pulse. A moving strong inductive electric field is generated inside of the target. We have successfully obtained a bunched ion beam in our particle-in-cell simulations in this paper.

  19. High temperature ion source for an on-line isotope separator

    DOEpatents

    Mlekodaj, Ronald L.

    1979-01-01

    A reduced size ion source for on-line use with a cyclotron heavy-ion beam is provided. A sixfold reduction in source volume while operating with similar input power levels results in a 2000.degree. C. operating temperature. A combined target/window normally provides the reaction products for ionization while isolating the ion source plasma from the cyclotron beam line vacuum. A graphite felt catcher stops the recoiling reaction products and releases them into the plasma through diffusion and evaporation. Other target arrangements are also possible. A twenty-four hour lifetime of unattended operation is achieved, and a wider range of elements can be studied than was heretofore possible.

  20. On-line estimation of laser-drilled hole depth using a machine vision method.

    PubMed

    Ho, Chao-Ching; He, Jun-Jia; Liao, Te-Ying

    2012-01-01

    The paper presents a novel method for monitoring and estimating the depth of a laser-drilled hole using machine vision. Through on-line image acquisition and analysis in laser machining processes, we could simultaneously obtain correlations between the machining processes and analyzed images. Based on the machine vision method, the depths of laser-machined holes could be estimated in real time. Therefore, a low cost on-line inspection system is developed to increase productivity. All of the processing work was performed in air under standard atmospheric conditions and gas assist was used. A correlation between the cumulative size of the laser-induced plasma region and the depth of the hole is presented. The result indicates that the estimated depths of the laser-drilled holes were a linear function of the cumulative plasma size, with a high degree of confidence. This research provides a novel machine vision-based method for estimating the depths of laser-drilled holes in real time.

  1. Laser ion source for high brightness heavy ion beam

    NASA Astrophysics Data System (ADS)

    Okamura, M.

    2016-09-01

    A laser ion source is known as a high current high charge state heavy ion source. However we place great emphasis on the capability to realize a high brightness ion source. A laser ion source has a pinpoint small volume where materials are ionized and can achieve quite uniform low temperature ion beam. Those features may enable us to realize very small emittance beams. In 2014, a low charge state high brightness laser ion source was successfully commissioned in Brookhaven National Laboratory. Now most of all the solid based heavy ions are being provided from the laser ion source for regular operation.

  2. On-Line Characterization of Gold Nanoparticles Generated by Laser Ablation in Liquids

    NASA Astrophysics Data System (ADS)

    Maciulevičius, M.; Vinčiūnas, A.; Brikas, M.; Butsen, A.; Tarasenka, N.; Tarasenko, N.; Račiukaitis, G.

    Size of nanoparticles is an important parameter for their applications. To develop the system for the on-line nanoparticle characterization during their production by a laser, the laser ablation chamber that allows measurement of the surface plasmon resonance spectra during nanoparticle generation process has been designed and fabricated. The mean diameter of nanoparticles was determined using their absorption spectra acquired in the real-time during the ablation experiments. The results were compared with the TEM images analysis and observed differences in size are discussed. The technique was applied to investigate the effect of additional laser irradiation on size distribution in gold colloids prepared by laser ablation in water and in aqueous glucose solution.

  3. First on-line results for As and F beams from HRIBF target/ion sources

    SciTech Connect

    Carter, H.K.; Kormicki, J.; Stracener, D.W.; Breitenbach, J.B.; Blackmon, J.C.; Smith, M.S.; Bardayan, D.W.

    1996-12-31

    The first on-line tests of the ion sources to provide radioactive ion beams of {sup 69,70}As and {sup 17,18}F for the Holifield Radioactive Ion Beam Facility have been performed using the UNISOR facility at HRIBF. For {sup 70}As the measured efficiency is 0.8 {+-} 0.3% with a hold-up time of 3.6 {+-} 0.3 hours as measured with {sup 72}As at a target temperature of 1,270 C. For {sup 17}F the efficiency for Al{sup 17}F is 0.0024 {+-} 0.0008% with a hold-up time of 16.4 {+-} 0.8 m as measured with Al{sup 18}F at a target temperature of 1,470 C.

  4. Resonant Ionization Laser Ion Source for Radioactive Ion Beams

    SciTech Connect

    Liu, Yuan; Beene, James R; Havener, Charles C; Vane, C Randy; Gottwald, T.; Wendt, K.; Mattolat, C.; Lassen, J.

    2009-01-01

    A resonant ionization laser ion source based on all-solid-state, tunable Ti:Sapphire lasers is being developed for the production of pure radioactive ion beams. It consists of a hot-cavity ion source and three pulsed Ti:Sapphire lasers operating at a 10 kHz pulse repetition rate. Spectroscopic studies are being conducted to develop ionization schemes that lead to ionizing an excited atom through an auto-ionization or a Rydberg state for numerous elements of interest. Three-photon resonant ionization of 12 elements has been recently demonstrated. The overall efficiency of the laser ion source measured for some of these elements ranges from 1 to 40%. The results indicate that Ti:Sapphire lasers could be well suited for laser ion source applications. The time structures of the ions produced by the pulsed lasers are investigated. The information may help to improve the laser ion source performance.

  5. On-line measurement of water-soluble ions in ambient particles

    NASA Astrophysics Data System (ADS)

    Wen, T. X.; Wang, Y. S.; Chang, S. Y.; Liu, G. R.

    2006-07-01

    Combining the system of rapid collection of ambient particles and ion chromatography, the system of rapid collection of fine particles and ion chromatography (RCFP-IC) was established to automatically analyze on-line the concentrations of water-soluble ions in ambient particles. Here, the general scheme SO42-, of RCFP-IC is described and its basic performance is tested. The detection limit of RCFP-IC for 4 NO3-, NO2-, Cl- and F- is below 0.3 mu g m(-3). The collection efficiency of RCFP-IC increases rapidly with increasing sized particles. For particles larger than 300 nm, the collection efficiency approaches 100%. The precision of RCFP-IC is more than 90% over 28 repetitions. The response of RCFP-IC is very sensitive and no obvious cross-pollution is found during measurement. A comparison of RCFP-IC with an integrated filter measurement indicates that the measurement of RCFP-IC is comparable in both laboratory experiments and field observations. The results of the field experiment prove that RCFP-IC is an effective on-line monitoring system and is helpful in source apportionment and pollution episode monitoring.

  6. Laser driven ion accelerator

    DOEpatents

    Tajima, Toshiki

    2006-04-18

    A system and method of accelerating ions in an accelerator to optimize the energy produced by a light source. Several parameters may be controlled in constructing a target used in the accelerator system to adjust performance of the accelerator system. These parameters include the material, thickness, geometry and surface of the target.

  7. On-line Raman spectroscopy of calcite and malachite during irradiation with swift heavy ions

    NASA Astrophysics Data System (ADS)

    Dedera, Sebastian; Burchard, Michael; Glasmacher, Ulrich A.; Schöppner, Nicole; Trautmann, Christina; Severin, Daniel; Romanenko, Anton; Hubert, Christian

    2015-12-01

    A new on-line Raman System, which was installed at the M3-beamline at the UNILAC, GSI Helmholtzzentrum für Schwerionenforschung Darmstadt was used for first "in situ" spectroscopic measurements. Calcite and malachite samples were irradiated in steps between 1 × 109 and 1 × 1012 ions/cm2 with Au ions (calcite) and Xe ions (malachite) at an energy of 4.8 MeV/u. After irradiation, calcite revealed a new Raman band at 437 cm-1 and change of the full width at half maximum for the 1087 cm-1 Raman band. The Raman bands of malachite change significantly with increasing fluence. Up to a fluence of 7 × 1010 ions/cm2, all existing bands decrease in intensity. Between 8 × 1010 and 1 × 1011 ions/cm2 a broad Cu2O band between 110 and 220 cm-1 occurs, which superimposes the pre-existing Raman bands. Additionally, a new broad band between 1000 and 1750 cm-1 is formed, which is interpreted as a carbon coating. In contrast to the Cu2O band, the carbon band vanished when further irradiating the sample. The installations as well as first in situ measurements at room temperature are presented.

  8. First on-line results for As and F beams from HRIBF target/ion sources

    SciTech Connect

    Stracener, D.W.; Carter, H.K.; Kormicki, J.; Breitenbach, J.B.; Blackmon, J.C.; Smith, M.S.; Bardayan, D.W.

    1996-12-31

    The first on-line tests of the ion sources to provide radioactive ion beams of {sup 69,70}As and {sup 17,18}F for the Holifield Radioactive Ion Beam Facility (HRIBF) have been performed using the UNISOR facility at HRIBF. The target/ion source is an electron beam plasma (EBP) source similar to the ISOLDE design. The measured efficiencies for {sup 69}As and {sup 70}AS were 0.5 {+-} 0.2% and 0.8 {+-} 0.3%, respectively. The arsenic hold-up time in the tested target ion source was 3.6 {+-} 0.3 hours as measured with {sup 72}As at a target temperature of 1300 {degrees}C. The measured efficiencies for {sup 17}F and {sup 18}F were 0.0052 {+-} 0.0008% and 0.06 {+-} 0.02%, respectively. The source hold-up time for fluorine was measured with Al{sup 18}F since 88% of the observed radioactive fluorine was found in this molecule. The Al{sup 18}F hold-up time was 16.4 {+-} 0.8 minutes at a target temperature of 1470 {degrees}C.

  9. Flash pyrolysis of coal by an argon ion laser

    SciTech Connect

    Thomsen, M.S.; Egsgaard, H.

    1994-12-31

    A novel approach to laser induced pyrolysis of coal by using the visible blue-green emission from an argon ion laser is presented. The gaseous pyrolysis products are identified by on-line gas chromatography/mass spectrometry (GC/MS). Five different subbituminous to bituminous coals have been studied and results for the low-molecular weight hydrocarbons up to C{sub 3} are discussed. Mechanisms for the formation of the unsaturated hydrocarbons, ethylene and acetylene, during laser pyrolysis of coal have been disclosed utilizing deuterium as a buffer gas in the pyrolysis cell.

  10. The beam diagnostic instruments in Beijing radioactive ion-beam facilities isotope separator on-line

    SciTech Connect

    Ma, Y. Cui, B.; Ma, R.; Tang, B.; Chen, L.; Huang, Q.; Jiang, W.

    2014-02-15

    The beam diagnostic instruments for Beijing Radioactive Ion-beam Facilities Isotope Separator On-Line are introduced [B. Q. Cui, Z. H. Peng, Y. J. Ma, R. G. Ma, B. Tang, T. Zhang, and W. S. Jiang, Nucl. Instrum. Methods 266, 4113 (2008); T. J. Zhang, X. L. Guan, and B. Q. Cui, in Proceedings of APAC 2004, Gyeongju, Korea, 2004, http://www.jacow.org , p. 267]. For low intensity ion beam [30–300 keV/1 pA–10 μA], the beam profile monitor, the emittance measurement unit, and the analyzing slit will be installed. For the primary proton beam [100 MeV/200 μA], the beam profile scanner will be installed. For identification of the nuclide, a beam identification unit will be installed. The details of prototype of the beam diagnostic units and some experiment results will be described in this article.

  11. Application of laser ultrasonic method for on-line monitoring of friction stir spot welding process.

    PubMed

    Zhang, Kuanshuang; Zhou, Zhenggan; Zhou, Jianghua

    2015-09-01

    Application of a laser ultrasonic method is developed for on-line monitoring of the friction stir spot welding (FSSW) process. Based on the technology of FSSW, laser-generated ultrasonic waves in a good weld and nonweld area are simulated by a finite element method. The reflected and transmitted waves are analyzed to disclose the properties of the welded interface. The noncontact-laser ultrasonic-inspection system was established to verify the numerical results. The reflected waves in the good-weld and nonweld area can be distinguished by time-of-flight. The transmitted waves evidently attenuate in the nonweld area in contrast to signal amplitude in the good weld area because of interfacial impedance difference. Laser ultrasonic C-scan images can sufficiently evaluate the intrinsic character of the weld area in comparison with traditional water-immersion ultrasonic testing results. The research results confirm that laser ultrasonics would be an effective method to realize the characterization of FSSW defects.

  12. A nanochannel based on-line universal logic ion sensing platform

    NASA Astrophysics Data System (ADS)

    Chen, Chaogui; Zhang, Xiaowei; Zhu, Jinbo; Li, Jing; Zhang, Libing; Wang, Erkang

    2013-08-01

    In this work, a novel ion sensing platform was constructed in a microfluidic chip based on a very easy nano-fabrication technique, with which the nanoscale channel generated along the junction of the PDMS and metal strip could serve as a salt bridge for electrochemical measurements. More importantly, we have proposed a flexible and universal ion sensing strategy based on Boolean logic, which can rapidly report the concentration of analyte by the approach method. Firstly, the performance of the nanochannel based salt bridge was characterized, and the results showed that the nanoscale salt bridge behaved comparably to the traditional ones. To illustrate the promising applications of this wonderful design, an IrOx electrode was employed to construct the on-line pH sensing device as an example, and a wide linearity range (pH 2-12) was obtained with a really high sensitivity of 74.15 mV per pH unit. Owing to the use of the logic sensing strategy, we achieved rapid identification of the sample pH on-line, and demonstrated the broad potential of our system in designing sensing devices with extremely high integration, automation and throughput.

  13. Agent-based station for on-line diagnostics by self-adaptive laser Doppler vibrometry.

    PubMed

    Serafini, S; Paone, N; Castellini, P

    2013-12-01

    A self-adaptive diagnostic system based on laser vibrometry is proposed for quality control of mechanical defects by vibration testing; it is developed for appliances at the end of an assembly line, but its characteristics are generally suited for testing most types of electromechanical products. It consists of a laser Doppler vibrometer, equipped with scanning mirrors and a camera, which implements self-adaptive bahaviour for optimizing the measurement. The system is conceived as a Quality Control Agent (QCA) and it is part of a Multi Agent System that supervises all the production line. The QCA behaviour is defined so to minimize measurement uncertainty during the on-line tests and to compensate target mis-positioning under guidance of a vision system. Best measurement conditions are reached by maximizing the amplitude of the optical Doppler beat signal (signal quality) and consequently minimize uncertainty. In this paper, the optimization strategy for measurement enhancement achieved by the down-hill algorithm (Nelder-Mead algorithm) and its effect on signal quality improvement is discussed. Tests on a washing machine in controlled operating conditions allow to evaluate the efficacy of the method; significant reduction of noise on vibration velocity spectra is observed. Results from on-line tests are presented, which demonstrate the potential of the system for industrial quality control.

  14. Agent-based station for on-line diagnostics by self-adaptive laser Doppler vibrometry

    NASA Astrophysics Data System (ADS)

    Serafini, S.; Paone, N.; Castellini, P.

    2013-12-01

    A self-adaptive diagnostic system based on laser vibrometry is proposed for quality control of mechanical defects by vibration testing; it is developed for appliances at the end of an assembly line, but its characteristics are generally suited for testing most types of electromechanical products. It consists of a laser Doppler vibrometer, equipped with scanning mirrors and a camera, which implements self-adaptive bahaviour for optimizing the measurement. The system is conceived as a Quality Control Agent (QCA) and it is part of a Multi Agent System that supervises all the production line. The QCA behaviour is defined so to minimize measurement uncertainty during the on-line tests and to compensate target mis-positioning under guidance of a vision system. Best measurement conditions are reached by maximizing the amplitude of the optical Doppler beat signal (signal quality) and consequently minimize uncertainty. In this paper, the optimization strategy for measurement enhancement achieved by the down-hill algorithm (Nelder-Mead algorithm) and its effect on signal quality improvement is discussed. Tests on a washing machine in controlled operating conditions allow to evaluate the efficacy of the method; significant reduction of noise on vibration velocity spectra is observed. Results from on-line tests are presented, which demonstrate the potential of the system for industrial quality control.

  15. Ion production from solid state laser ion sources

    SciTech Connect

    Gottwald, T.; Mattolat, C.; Raeder, S.; Wendt, K.; Havener, C.; Liu, Y.; Lassen, J.; Rothe, S.

    2010-02-15

    Laser ion sources based on resonant excitation and ionization of atoms are well-established tools for selective and efficient production of radioactive ion beams. Recent developments are focused on the use of the state-of-the-art all solid-state laser systems. To date, 35 elements of the periodic table are available from laser ion sources based on tunable Ti:sapphire lasers. Recent progress in this field regarding the establishment of suitable optical excitation schemes for Ti:sapphire lasers are reported.

  16. On-line wavelength calibration of pulsed laser for CO2 DIAL sensing

    NASA Astrophysics Data System (ADS)

    Han, Ge; Gong, Wei; Lin, Hong; Ma, Xin; Xiang, Chengzhi

    2014-12-01

    Accurate on-line wavelength calibration is a crucial procedure for sensing atmospheric CO2 using the DIAL technique. Drastic fluctuations in the intensity of a pulsed laser pose a great challenge for accurate on-line wavelength determination and stabilization, resulting in CO2 retrievals lacking the desired accuracy for global climate change and carbon cycle research. To tackle this problem, a two-stage wavelength calibration method based on Voigt fitting was proposed in this work. Simulation analysis demonstrated that the proposed method is superior to the conventional method and provides wavelength calibration results with an accuracy of 0.1 pm when the noise level does not exceed than 5 %. This conclusion was confirmed through experiments with real signals. Furthermore, simulation analysis revealed that the proposed method could yield results with an accuracy of 0.1 pm by increasing the number of sample points, even for signals with noise levels of up to 20 %. This is a promising feature that could facilitate the development of DIAL systems without gas cells.

  17. A novel health indicator for on-line lithium-ion batteries remaining useful life prediction

    NASA Astrophysics Data System (ADS)

    Zhou, Yapeng; Huang, Miaohua; Chen, Yupu; Tao, Ye

    2016-07-01

    Prediction of lithium-ion batteries remaining useful life (RUL) plays an important role in an intelligent battery management system. The capacity and internal resistance are often used as the batteries health indicator (HI) for quantifying degradation and predicting RUL. However, on-line measurement of capacity and internal resistance are hardly realizable due to the not fully charged and discharged condition and the extremely expensive cost, respectively. Therefore, there is a great need to find an optional way to deal with this plight. In this work, a novel HI is extracted from the operating parameters of lithium-ion batteries for degradation modeling and RUL prediction. Moreover, Box-Cox transformation is employed to improve HI performance. Then Pearson and Spearman correlation analyses are utilized to evaluate the similarity between real capacity and the estimated capacity derived from the HI. Next, both simple statistical regression technique and optimized relevance vector machine are employed to predict the RUL based on the presented HI. The correlation analyses and prediction results show the efficiency and effectiveness of the proposed HI for battery degradation modeling and RUL prediction.

  18. Laser ion source with solenoid field

    SciTech Connect

    Kanesue, Takeshi; Fuwa, Yasuhiro; Kondo, Kotaro; Okamura, Masahiro

    2014-11-12

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. In this study, the laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 1011, which was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.

  19. Laser ion source with solenoid field

    DOE PAGES

    Kanesue, Takeshi; Fuwa, Yasuhiro; Kondo, Kotaro; Okamura, Masahiro

    2014-11-12

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. In this study, the laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 1011, whichmore » was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.« less

  20. Laser ion source with solenoid field

    SciTech Connect

    Kanesue, Takeshi Okamura, Masahiro; Fuwa, Yasuhiro; Kondo, Kotaro

    2014-11-10

    Pulse length extension of highly charged ion beam generated from a laser ion source is experimentally demonstrated. The laser ion source (LIS) has been recognized as one of the most powerful heavy ion source. However, it was difficult to provide long pulse beams. By applying a solenoid field (90 mT, 1 m) at plasma drifting section, a pulse length of carbon ion beam reached 3.2 μs which was 4.4 times longer than the width from a conventional LIS. The particle number of carbon ions accelerated by a radio frequency quadrupole linear accelerator was 1.2 × 10{sup 11}, which was provided by a single 1 J Nd-YAG laser shot. A laser ion source with solenoid field could be used in a next generation heavy ion accelerator.

  1. A test stand for off-line laser ion source development at TRIUMF

    SciTech Connect

    Lavoie, J. P.; Li, R.; Bricault, P.; Lassen, J.; Chachkova, O.; Teigelhoefer, A.

    2013-01-15

    A test stand for ion source development and laser resonance ionization spectroscopy was built and commissioned at TRIUMF. The test stand is needed to develop efficient ion sources that can function reliably in the hostile, high temperature, high radiation environment of TRIUMF's isotope separator on-line (ISOL) production target ion source. In addition, it enables laser resonance ionization spectroscopy to develop laser excitation schemes suitable for the solid-state laser systems used with TRIUMF's resonant ionization laser ion source . Also, it allows for possible improvement of current ion sources and validation of new designs. The test stand employs a copy of the ion optics used on-line, so that results can be transferred directly to radioactive ion beam production. Due to space restrictions and the need for rapid mass scans, a quadrupole mass spectrometer is used as a mass separator. One of the first experiments conducted on the laser ion source test stand (LIS STAND) was resonant ionization spectroscopy of gallium to improve on the ionization scheme previously used on-line, so that low yield isotopes (e.g., {sup 62}Ga) become available for experiments. Different Rydberg series in gallium were observed and autoionizing states were searched for. The overall LIS STAND system performance, characteristics, and the first resonant ionization spectroscopy are described.

  2. Bacterial cells enhance laser driven ion acceleration

    PubMed Central

    Dalui, Malay; Kundu, M.; Trivikram, T. Madhu; Rajeev, R.; Ray, Krishanu; Krishnamurthy, M.

    2014-01-01

    Intense laser produced plasmas generate hot electrons which in turn leads to ion acceleration. Ability to generate faster ions or hotter electrons using the same laser parameters is one of the main outstanding paradigms in the intense laser-plasma physics. Here, we present a simple, albeit, unconventional target that succeeds in generating 700 keV carbon ions where conventional targets for the same laser parameters generate at most 40 keV. A few layers of micron sized bacteria coating on a polished surface increases the laser energy coupling and generates a hotter plasma which is more effective for the ion acceleration compared to the conventional polished targets. Particle-in-cell simulations show that micro-particle coated target are much more effective in ion acceleration as seen in the experiment. We envisage that the accelerated, high-energy carbon ions can be used as a source for multiple applications. PMID:25102948

  3. Quality control agent: Self-adaptive laser vibrometry for on-line diagnostics

    NASA Astrophysics Data System (ADS)

    Serafini, S.; Paone, N.; Castellini, P.

    2012-06-01

    It is presented the development of a self-adaptive diagnostic system based on laser vibrometry for production line quality control. The vibration measurement system consists of a laser Doppler vibrometer, equipped with scanning mirrors and a smart camera, which implements self-adaptivity for compensating target mis-positioning under guidance by a vision system and for the achievement of the best condition for measurement by optimizing the Doppler signal level. This system is designed as a Quality Control Agent (QCA) and it is part of a Multi Agent System (MAS) that supervises all the production line. The QCA behavior is defined so to perform a minimization of measurement uncertainty during the on line tests; for this purpose the QCA exhibits a self-adaptive behavior. Best measurement conditions are defined in terms of amplitude of the optical Doppler beat signal (signal quality - SQ). In this paper, the optimization strategy for measurement enhancement achieved by the down-hill algorithm (Nelder-Mead algorithm) and its effect on signal quality improvement is discussed. Tests on a washing machine in controlled operating conditions allow to evaluate the efficacy of the method; significant reduction of noise on vibration velocity spectra is observed.

  4. TITAN: An ion trap facility for on-line mass measurement experiments

    NASA Astrophysics Data System (ADS)

    Kwiatkowski, A. A.; Andreoiu, C.; Bale, J. C.; Brunner, T.; Chaudhuri, A.; Chowdhury, U.; Delheij, P.; Ettenauer, S.; Frekers, D.; Gallant, A. T.; Grossheim, A.; Gwinner, G.; Jang, F.; Lennarz, A.; Ma, T.; Mané, E.; Pearson, M. R.; Schultz, B. E.; Simon, M. C.; Simon, V. V.; Dilling, J.

    2014-01-01

    Precision determinations of ground state or even isomeric state masses reveal fingerprints of nuclear structure. In particular, at the limits of existence for very neutron-rich or -deficient isotopes, one can extract detailed information about nuclear structure from separation energies or binding energies. Mass measurements are important to uncover new phenomena, to test new theoretical predictions, or to refine model approaches. For example, the N = 28 shell has proven more stable than previously expected; however, the predicted new "magic" number at N = 34 in the K and Ca isotopes has yet to be confirmed experimentally. For these neutron-rich nuclei, the inclusion of three-body forces leads to significantly better predictions of the ground-state mass. Similarly, halo nuclei present an excellent application for ab-initio theory, where ground state properties, like masses and radii, test our understanding of nuclear structure. Precision mass determinations at TRIUMF are carried out with the TITAN (TRIUMF's Ion Traps for Atomic and Nuclear science) facility. It is an ion-trap setup coupled to the on-line facility ISAC. TITAN has measured masses of isotopes as short-lived as 9 ms (almost an order of magnitude shorter-lived than any other Penning trap system), and it is the only one with charge breeding capabilities, which allow us to boost the precision by almost 2 orders of magnitude. We recently made use of this feature by measuring short-lived, proton-rich Rb-isotopes, up to 74Rb while reaching the 12 + charge state, which together with other improvements led to an increase in precision by a factor 36.

  5. The Resonance Laser Ion Source at Ipn-Atlo

    NASA Astrophysics Data System (ADS)

    Li, R.; Franchoo, S.; Lau, C.; Fedosseev, V.; Goodacre, T. D.; March, B.; Flanagan, K.; Kron, T.; Wendt, K.

    2015-06-01

    Resonant Ionization Laser Ion Source (RILIS), based on the stepwise excitations of atomic transitions, offers an outstanding combination of excellent elemental selectivity and high ionization efficiency. It has become a powerful and versatile tool for generation of pure radioactive isotope beams at on-line mass separator facilities worldwide. Initiated in 2009, IPN-Orsay has installed RILIS in the Isotope Separators on-line (ISOL) system at the photofission facility ALTO, which aims to the measurements of the nuclear properties of exotic nuclei through β-γ and β-n spectroscopy, among other techniques. RILS at ALTO (RIALTO) consists of two dye lasers pumped with a 532nm 10kHz Nd:YAG laser with the wavelength extension options via frequency doubling/tripling of nonlinear crystals. Gallium and Zinc isotopic beams were successfully delivered by RIALTO starting from 2011. To develop the laser ionization scheme for different elements and test optimal operational parameters for on-line radioactive beam deliveries, an off-line reference cell has been built. The preliminary result of the first commence of the off-line reference cell will be presented in this paper.

  6. Ion temperature via laser scattering on ion Bernstein waves

    SciTech Connect

    Wurden, G.A.; Ono, M.; Wong, K.L.

    1981-10-01

    Hydrogen ion temperature has been measured in a warm toroidal plasma with externally launched ion Bernstein waves detected by heterodyne CO/sub 2/ laser scattering. Radial scanning of the laser beam allows precise determination of k/sub perpendicular to/ for the finite ion Larmor radius wave (..omega.. approx. less than or equal to 2..cap omega../sub i/). Knowledge of the magnetic field strength and ion concentration then give a radially resolved ion temperature from the dispersion relation. Probe measurements and Doppler broadening of ArII 4806A give excellent agreement.

  7. On Line Characterization of SiC Nanoparticles Produced by Laser Pyrolysis

    NASA Astrophysics Data System (ADS)

    Wattieaux, G.; Lecerf, P.; Meyer, L.; Boufendi, L.; Leconte, Y.; Sublemontier, O.; Herlin, N.; Asimakopoulou, A.; Tsakis, A.; Daskalos, M.; Konstandopoulos, A. G.; Ouf, F. X.

    2011-07-01

    On Line Measurements campaigns have been carried out for the first time in IRAMIS/SPAM CEA's laser gas-phase pyrolysis nanoparticles production facilities. The produced aerosol is composed of Argon and/or Helium laden with SiC nanoparticles concentrated up to ~14 mg/l. Different commercial apparatus were used for sampling, and characterisation of size, and morphology of the particles. A series of experiment is performed by IRSN with a DMS500 from Cambustion Ltd™, which gives electrical mobility equivalent diameter distribution in real time. Particles are sampled with an ejector-diluter VKL-10 from Palas™. On the same sampling line, APTL performed aerodynamic equivalent diameter mass distribution using a Nanomoudi from MSP Corp.™ and TEM post analysis, as well as post elemental analysis (EDS) after collection on TEM grid with a Thermophoretic Precipitator (TP). A previously developed model is used to obtain the aggregate morphology and primary particles sizes. In addition to these commercial or well-known techniques, a new patent-pending technique called RFPM (Radio Frequency Plasma Metrology developed by CILAS + GREMI in the frame of NANOCARA program) is tested for the first time off the lab. The principle is based on levitation of particles in plasma RF. The entire set up is a prototype, including the sampling line. Experiments showed that this technique is very promising for on line gas phase monitoring, even though future improvements are needed, especially on the direct injection of the sample in the measuring chamber. First results of size distribution on pyrolysis line were obtained: three modes of different geometric mean diameter D50 were measured. Further analysis of TEM micrographs gave insight on these three modes, they can be interpreted as primary particles, aggregated particles, and a third one which could be composed of silica oxide nanoparticles issued from the combustion of the remaining silane initiated by an air leak in the exhaust of the

  8. Ion implantation and laser annealing

    NASA Astrophysics Data System (ADS)

    Three ion implantation and laser annealing projects have been performed by ORNL through the DOE sponsored Seed Money Program. The research has contributed toward improving the characteristics of wear, hardness, and corrosion resistance of some metals and ceramics, as well as the electrical properties of semiconductors. The work has helped to spawn related research, at ORNL and elsewhere, concerning the relationships between microstructure and materials properties. ORNL research has resulted in major advances in extended life and non-corrosive artificial joints (hip and knee), high performance semiconductors, failure resistant ceramics (with potential energy applications), and solar cells. The success of the seed money projects was instrumental in the formation of ORNL's Surface Modification and Characterization Facility (SMAC). More than 60 universities and companies have participated in SMAC programs.

  9. Laser-cooled atomic ions as probes of molecular ions

    SciTech Connect

    Brown, Kenneth R.; Viteri, C. Ricardo; Clark, Craig R.; Goeders, James E.; Khanyile, Ncamiso B.; Vittorini, Grahame D.

    2015-01-22

    Trapped laser-cooled atomic ions are a new tool for understanding cold molecular ions. The atomic ions not only sympathetically cool the molecular ions to millikelvin temperatures, but the bright atomic ion fluorescence can also serve as a detector of both molecular reactions and molecular spectra. We are working towards the detection of single molecular ion spectra by sympathetic heating spectroscopy. Sympathetic heating spectroscopy uses the coupled motion of two trapped ions to measure the spectra of one ion by observing changes in the fluorescence of the other ion. Sympathetic heating spectroscopy is a generalization of quantum logic spectroscopy, but does not require ions in the motional ground state or coherent control of the ion internal states. We have recently demonstrated this technique using two isotopes of Ca{sup +} [Phys. Rev. A, 81, 043428 (2010)]. Limits of the method and potential applications for molecular spectroscopy are discussed.

  10. Laser ion source for isobaric heavy ion collider experiment.

    PubMed

    Kanesue, T; Kumaki, M; Ikeda, S; Okamura, M

    2016-02-01

    Heavy-ion collider experiment in isobaric system is under investigation at Relativistic Heavy Ion Collider. For this experiment, ion source is required to maximize the abundance of the intended isotope. The candidate of the experiment is (96)Ru + (96)Zr. Since the natural abundance of particular isotope is low and composition of isotope from ion source depends on the composites of the target, an isotope enriched material may be needed as a target. We studied the performance of the laser ion source required for the experiment for Zr ions.

  11. On-line depth measurement for laser-drilled holes based on the intensity of plasma emission

    NASA Astrophysics Data System (ADS)

    Ho, Chao-Ching; Chiu, Chih-Mu; Chang, Yuan-Jen; Hsu, Jin-Chen; Kuo, Chia-Lung

    2014-09-01

    The direct time-resolved depth measurement of blind holes is extremely difficult due to the short time interval and the limited space inside the hole. This work presents a method that involves on-line plasma emission acquisition and analysis to obtain correlations between the machining processes and the optical signal output. Given that the depths of laser-machined holes can be estimated on-line using a coaxial photodiode, this was employed in our inspection system. Our experiments were conducted in air under normal atmospheric conditions without gas assist. The intensity of radiation emitted from the vaporized material was found to correlate with the depth of the hole. The results indicate that the estimated depths of the laser-drilled holes were inversely proportional to the maximum plasma light emission measured for a given laser pulse number.

  12. On-line cation exchange for suppression of adduct formation in negative-ion electrospray mass spectrometry of nucleic acids.

    PubMed

    Huber, C G; Buchmeiser, M R

    1998-12-15

    One major difficulty in the analysis of nucleic acids by electrospray mass spectrometry is represented by the affinity of the polyanionic sugar-phosphate backbone for nonvolatile cations, especially ubiquitous sodium and potassium ions. A simple on-line sample preparation system comprising a microflow pumping system and 45 x 0.8-mm-i.d. microcolumns packed with weak or strong cation-exchange resins is described for the efficient removal of cations from nucleic acid samples. Samples were analyzed by flow injection analysis at a 3-5 microL/min flow of 10 mM triethylamine in 50% water-50% acetonitrile. After on-line desalting, mass spectra of oligonucleotides revealed no significant sodium adduct peaks. Moreover, signal-to-noise ratios were greatly enhanced compared to direct injection of the samples. Electrospray mass spectrometry with on-line sample preparation allowed accurate molecular mass determinations of picomole amounts of crude oligonucleotide preparations ranging in size from 8 to 80 nucleotides within a few minutes. The good linearity of the calibration plot (R2 = 0.9988) over at least 2 orders of magnitude and a relative standard deviation in peak areas of less than 9% permitted the sensitive quantitative measurement of oligonucleotides in a concentration range of 0.2-20 microM with selected-ion monitoring. Finally, the on-line sample preparation system was evaluated for the mass spectrometric analysis of complex oligonucleotide mixtures. PMID:9868919

  13. On-line reaction monitoring in the liquid phase using two mid-infrared quantum cascade lasers simultaneously.

    PubMed

    Schaden, Stefan; Domínguez-Vidal, Ana; Lendl, Bernhard

    2006-05-01

    On-line monitoring of a model reaction was performed by employing two pulsed mid-infrared Fabry-Pérot quantum cascade lasers (QCL). The emission maxima of the QCLs were located at 1393 and 1080 cm(-1). An optical system of parabolic mirrors and a ZnSe beam splitter combined the two laser beams and allowed a transmission cell to be probed with both QCLs simultaneously. The reaction mixture was pumped continuously through a cell that had an optical path of 48 microm. This dual QCL system allowed fast absorption measurements of the reaction mixture at two distinct wavenumbers. The reaction under study was the oxidation of sulfite to sulfate with hydrogen peroxide acting as oxidant. On-line measurements of the chemical reaction allowed direct, real-time monitoring of sulfate formation and hydrogen peroxide depletion.

  14. Analysis of hexavalent chromium in Colla corii asini with on-line sample pretreatment valve-switching ion chromatography.

    PubMed

    Yang, Yuling; He, Jie; Huang, Zhongping; Zhong, Naifei; Zhu, Zuoyi; Jiang, Renyu; You, Jinghua; Lu, Xiuyang; Zhu, Yan; He, Shiwei

    2013-08-30

    An ion chromatography (IC) system with on-line sample pretreatment using valve-switching technique was developed for the determination of hexavalent chromium (Cr(VI)) in Colla corii asini. Colla corii asini is a complicated sample with organics as main matrix. In this work, a polymer-based reversed-phase column was used as a pretreatment column. Via valve-switching technique, sample solution with target ions were eluted from a collection loop to analytical columns, with matrix eliminated on-line. Under the optimized separation conditions, the method showed good linearity (r=0.9998) in the range of 0.004-1.0mg/L and satisfactory repeatability (RSD<3%, n=6). The limit of detection (LOD) was 1.4μg/L (S/N=3). The average spiked recoveries of Cr(VI) were 93.4-102.0%. The result showed that the on-line sample pretreatment IC system was convenient and practical for the determination of trace Cr(VI) in Colla corii asini samples.

  15. [Simultaneous determination of 16 organic acids in feed additives by on-line enrichment and ion chromatography-mass spectrometry].

    PubMed

    Xiong, Zhiyu; Dong, Ying; Zhou, Hongbin; Yu, Yang; Li, Jing; Sun, Li

    2014-02-01

    A novel analytical method for simultaneous determination of sixteen organic acids by on-line enrichment and ion chromatography-mass spectrometry (IC-MS) was developed. Online enrichment and separation of the organic acids were performed by ion chromatography on a homemade enrichment column and a homemade separation column. The qualitative and quantitative analyses of the organic acids were performed by mass spectrometry in selected ion monitoring (SIM) mode on the basis of atmospheric pressure chemical ionization (APCI) source in negative mode. The sample of 200 microL was injected for the analysis, and the on-line enrichment time was 3 min. The sodium hydroxide solution was used as a gradient elution system. The two columns made it possible to have a low limit of detection due to the good enrichment and separation capability. The sixteen organic acids were separated completely within 30 min. All curves showed good linearity within the test concentration ranges. The limits of detection (LODs) were between 0.01 and 0.22 mg/L, and the average recoveries were between 70.6% and 110.8%. The relative standard deviations (RSDs) were less than 6.3%. The results indicate that this method is simple, rapid, sensitive and accurate for the determination of the organic acids in feed additives.

  16. Possibilities of research for on-line mass separator with heavy ion reactions

    NASA Astrophysics Data System (ADS)

    Siváček, I.; Kliman, J.; Rodin, A. M.; Krupa, L'; Belozerov, A. V.; Podshibyakin, A. V.; Salamatin, V. S.; Stepantsov, S. V.; Vedeneev, V. Yu

    2014-09-01

    Mass Analyser of Superheavy Atoms is ISOL - type setup created for direct mass measurement heavy ions. Hot catcher and ECR ion source combination allows effective formation of secondary beams of volatile elements. Powerful magnetic analysing system offers possibility to achieve mass resolution M/ΔM > 1000 in the focal plane silicon strip detector. The efficiency, time characteristics and detection system properties are described. Two applications of setup in different fields of research are presented together with methodology of experiments and data analysis.

  17. ON-LINE ANALYSIS OF AQUEOUS AEROSOLS BY LASER DESORPTION IONIZATION. (R823980)

    EPA Science Inventory

    In this work the effects of water on the laser desorption ionization mass spectra of single aerosol particles are explored. Aqueous aerosols are produced by passing dry particles through a humid environment so that they undergo deliquescent growth. Laser desorption ionization is ...

  18. On-line gas-free electrodialytic eluent generator for capillary ion chromatography.

    PubMed

    Yang, Bingcheng; Takeuchi, Masaki; Dasgupta, Purnendu K

    2008-01-01

    Both low- and high-pressure, gas-free, capillary-scale electrodialytic generators for eluents in ion chromatography are described. While the low-pressure devices rely on planar or tubular membranes, the high-pressure devices rely on ion-exchange beads used both as one-way ionic gates and as ball-on-seat valves to provide sealing. The high-pressure device is easily implemented in the form of a commercial cross fitting and can withstand at least 1400 psi. By design these devices do not produce gas in the eluent channel; hence, it is not necessary to remove gas afterward. With appropriate electrolytes and electrode polarities, such devices can produce either acid or base or salt. In regard to ionic transport, the behavior of these devices fully corresponds to that of a semiconductor diode. To our knowledge, this is the first time such complete equivalence of ion transport through ion-exchange media and with the more familiar example of electron transport through a semiconductor diode under both forward- and reverse-biased conditions have been demonstrated. Reverse bias can be applied to minimize/prevent Donnan-forbidden leakage or ion exchange. Even with 4 M KOH in the electrode compartments and 4 microL/min water flowing through the eluent channel, with a reverse bias of -12 V, the leakage KOH concentration is <30 microM, whereas the KOH concentration with zero voltage applied, herein after termed open circuit penetration (OCP), is 1600 microM. It is suggested that this OCP occurs not as much through Donnan-forbidden leakage but via ion exchange. Chromatograms and reproducibility data are presented for both isocratic and gradient chromatography, using ion-exchange, latex-modified, open tubular and packed monolithic columns.

  19. Ion beam control in laser plasma interaction

    NASA Astrophysics Data System (ADS)

    Kawata, S.; Izumiyama, T.; Sato, D.; Nagashima, T.; Takano, M.; Barada, D.; Gu, Y. J.; Ma, Y. Y.; Kong, Q.; Wang, P. X.; Wang, W. M.

    2016-03-01

    By a two-stage successive acceleration in laser ion acceleration, our 2.5-dimensional particle-in-cell simulations demonstrate a remarkable increase in ion energy by a few hundreds of MeV; the maximum proton energy reaches about 250MeV. The ions are accelerated by the inductive continuous post-acceleration in a laser plasma interaction together with the target normal sheath acceleration and the breakout afterburner mechanism. An intense short-pulse laser generates a strong current by high-energy electrons accelerated, when an intense short- pulse laser illuminates a plasma target. The strong electric current creates a strong magnetic field along the high-energy electron current in the plasma. During the increase phase in the magnetic field strength, the moving longitudinal inductive electric field is induced by the Faraday law, and accelerates the forward-moving ions continously. The multi-stage acceleration provides a unique controllability in the ion energy and its quality.

  20. Proton emission from a laser ion source

    SciTech Connect

    Torrisi, L.; Cavallaro, S.; Gammino, S.; Cutroneo, M.; Margarone, D.

    2012-02-15

    At intensities of the order of 10{sup 10} W/cm{sup 2}, ns pulsed lasers can be employed to ablate solid bulk targets in order to produce high emission of ions at different charge state and kinetic energy. A special interest is devoted to the production of protons with controllable energy and current from a roto-translating target irradiated in repetition rate at 1-10 Hz by a Nd:Yag pulsed laser beam. Different hydrogenated targets based on polymers and hydrates were irradiated in high vacuum. Special nanostrucutres can be embedded in the polymers in order to modify the laser absorption properties and the amount of protons to be accelerated in the plasma. For example, carbon nanotubes may increase the laser absorption and the hydrogen absorption to generate high proton yields from the plasma. Metallic nanostrucutres may increase the electron density of the plasma and the kinetic energy of the accelerated protons. Ion collectors, ion energy analyzer, and mass spectrometers, used in time-of-flight configuration, were employed to characterize the ion beam properties. A comparison with traditional proton ion source is presented and discussed.

  1. Ion laser isotope enrichment by photo-predissociation of formaldehyde

    DOEpatents

    Marling, John B.

    1977-06-17

    Enrichment of carbon, hydrogen and/or oxygen isotopes by means of isotopically selective photo-predissociation of formaldehyde is achieved by irradiation with a fixed frequency ion laser, specifically, a neon, cadmium, or xenon ion laser.

  2. Laser-driven inertial ion focusing.

    PubMed

    Zhuo, H B; Yu, Wei; Yu, M Y; Xu, H; Wang, X; Shen, B F; Sheng, Z M; Zhang, J

    2009-01-01

    A Hohlraum-like configuration is proposed for realizing a simple compact source for neutrons. A laser pulse enters a tiny thin-shelled hollow-sphere target through a small opening and is self-consistently trapped in the cavity. The electrons in the inner shell-wall region are expelled by the light pressure. The resulting space-charge field compresses the local ions into a thin layer that becomes strongly heated. An inward expansion of ions into the shell cavity then occurs, resulting in the formation at the cavity center of a hot spot of ions at high density and temperature, similar to that in inertial electrostatic confinement.

  3. Laser-induced fluorescence method for on-line molecular isotopologues of iodine-127, iodine-129, iodine-131 detected in gaseous media using a tunable diode laser

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Shnyrev, S. L.; Sobolevsky, I. V.

    2016-06-01

    The letter reports on the development of a laser-induced fluorescence method for on-line selective measurement of 127I2, 129I2, 131I2, 129I127I, 127I131I, 129I131I isotopologue concentrations in gaseous media. The method is based on the excitation of molecular iodine isotopologues’ fluorescence by tunable diode laser (632–637 nm) radiation at three or four wavelengths corresponding to the 127I2, 131I2, 129I127I, 129I131I absorption line centers. Boundary relations for concentrations of simultaneously measured iodine isotopologues is about 10‑5–10‑6.

  4. “Development of an Automated On-line Electrochemical Chlorite Ion Sensor”

    PubMed Central

    Myers, John N.; Steinecker, William H.; Sandlin, Zechariah D.; Cox, James A.; Gordon, Gilbert; Pacey, Gilbert E.

    2012-01-01

    A sensor system for the automatic, in-line, determination of chlorite ion is reported. Electroanalytical measurements were performed in electrolyte-free liquids by using an electrochemical probe (EC), which enables in-line detection in high-resistance media such as disinfected water. Cyclic voltammetry scan rate studies suggest that the current arising from the oxidation of chlorite ion at an EC probe is mass-transfer limited. By coupling FIA with an EC probe amperometric cell, automated analysis was achieved. This sensor is intended to fulfill the daily monitoring requirements of the EPA DBP regulations for chlorite ion. Detection limits of 0.02-0.13 mg/L were attained, which is about one order of magnitude below the MRDL. The sensor showed no faradaic signal for perchlorate, chlorate, or nitrate. The lifetime and stability of the sensor were investigated by measuring calibration curves over time under constant-flow conditions. Detection limits of <0.1 mg/L were repeatedly achieved over a period of three weeks. PMID:22608440

  5. Laser photoelectron spectroscopy of ions

    SciTech Connect

    Ellison, G.B.

    1993-12-01

    During the last year the author has (a) completed a review article that critically contrasts three methods to measure R-H bond energies, (b) finished a spectroscopic study of the phenylnitrene anion, and (c) successfully completed an overhaul of the light source of the photodetachment spectrometer. The new light source is based on an Ar III laser that provides approximately 100 W of 3.531 eV photons.

  6. Oncological hadrontherapy with laser ion accelerators

    NASA Astrophysics Data System (ADS)

    Bulanov, S. V.; Esirkepov, T. Zh.; Khoroshkov, V. S.; Kuznetsov, A. V.; Pegoraro, F.

    2002-11-01

    === Effective ion acceleration during the interaction of an ultra short and ultra intense laser pulse with matter is one of the most important applications of the presently available compact laser systems with multi-terawatt and petawatt power. The use of an intense collimated beam of protons produced by a high-intensity laser pulse interacting with a plasma for the proton treatment of oncological diseases [1,2] is discussed. The fast proton beam is produced at the target by direct laser acceleration. An appropriately designed double-layer target scheme is proposed in order to achieve high-quality proton beams. The generation of high quality proton beams is proved with Particle in Cell simulations. === [1] S. V. Bulanov, V. S. Khoroshkov, Plasma Phys. Rep. 28, 453 (2002). [2] S. V. Bulanov, T. Zh. Esirkepov, V. S. Khoroshkov, A.V. Kuznetsov, F. Pegoraro, Phys. Lett. A 299, 240 (2002)

  7. On-line computer system to minimize laser injuries during surgery: preliminary system layout and proposal of the key features.

    PubMed

    Canestri, F

    1999-01-01

    The aim of this paper is to investigate some new user interface ideas and related application packages which aim to improve the degree of safety in an operating room during surgical operations in which an invasive laser beam is deployed. The overall value of the proposition is that a means is provided which ensures the successful completion of the surgical case while minimizing the risk of thermal and mechanical injuries to healthy tissues adjacent to the surgical field. According to surgeons operating with a variety of CO2 lasers available at both the National Cancer Institute in Milan, Italy, and the Sackler School of Medicine, Tel Aviv University, Israel, each laser device presents different cutting and coagulation properties. In order to identify which 'ideal' procedure might corroborate the subjective impression of each surgeon and also to provide one common tool to ensure procedures with a high level of safety, the author has worked for several months with surgeons and technicians of both Institutions to define the general design of a new on-line surgical operation planning and design system to be used during the pre-operative briefing activities and also as a consultation tool during operation. This software package will be developed and tested on both 'C' and FORTRAN compilers running on a commercially available PC which is driving a continuous wave (CW) CO2 laser device via its Instrument Bus interface. The present proposal describes the details of a software package called LCA (Laser-beam Controller and Adviser) which performs several controls in parallel on the key output parameters of a laser beam device during its utilization in delicate surgical operations. The required performances of this device needed during a given surgical operation are pre-simulated and compared against the well-known safety limits, which are stored in the computer's mass storage. If the surgeon's decision about the laser device set-up are considered to be too close to the

  8. Controllability in Multi-Stage Laser Ion Acceleration

    NASA Astrophysics Data System (ADS)

    Kawata, S.; Kamiyama, D.; Ohtake, Y.; Barada, D.; Ma, Y. Y.; Kong, Q.; Wang, P. X.; Gu, Y. J.; Li, X. F.; Yu, Q.

    2015-11-01

    The present paper shows a concept for a future laser ion accelerator, which should have an ion source, ion collimators, ion beam bunchers and ion post acceleration devices. Based on the laser ion accelerator components, the ion particle energy and the ion energy spectrum are controlled, and a future compact laser ion accelerator would be designed for ion cancer therapy or for ion material treatment. In this study each component is designed to control the ion beam quality. The energy efficiency from the laser to ions is improved by using a solid target with a fine sub-wavelength structure or a near-critical density gas plasma. The ion beam collimation is performed by holes behind the solid target or a multi-layered solid target. The control of the ion energy spectrum and the ion particle energy, and the ion beam bunching are successfully realized by a multi-stage laser-target interaction. A combination of each component provides a high controllability of the ion beam quality to meet variable requirements in various purposes in the laser ion accelerator. The work was partly supported by MEXT, JSPS, ASHULA project/ ILE, Osaka University, CORE (Center for Optical Research and Education, Utsunomiya University, Japan), Fudan University and CDI (Creative Dept. for Innovation) in CCRD, Utsunomiya University.

  9. A laser ablation source for offline ion production at LEBIT

    NASA Astrophysics Data System (ADS)

    Izzo, C.; Bollen, G.; Bustabad, S.; Eibach, M.; Gulyuz, K.; Morrissey, D. J.; Redshaw, M.; Ringle, R.; Sandler, R.; Schwarz, S.; Valverde, A. A.

    2016-06-01

    A laser ablation ion source has been developed and implemented at the Low-Energy Beam and Ion Trap (LEBIT) facility at the National Superconducting Cyclotron Laboratory. This offline ion source enhances the capabilities of LEBIT by providing increased access to ions used for calibration measurements and checks of systematic effects as well as stable and long-lived ions of scientific interest. The design of the laser ablation ion source and a demonstration of its successful operation are presented.

  10. Biomonitoring of essential and toxic metals in single hair using on-line solution-based calibration in laser ablation inductively coupled plasma mass spectrometry.

    PubMed

    Dressler, Valderi L; Pozebon, Dirce; Mesko, Marcia Foster; Matusch, Andreas; Kumtabtim, Usarat; Wu, B; Sabine Becker, J

    2010-10-15

    Laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) has been established as a powerful and sensitive surface analytical technique for the determination of concentration and distribution of trace metals within biological systems at micrometer spatial resolution. LA-ICP-MS allows easy quantification procedures if suitable standard references materials (SRM) are available. In this work a new SRM-free approach of solution-based calibration method in LA-ICP-MS for element quantification in hair is described. A dual argon flow of the carrier gas and nebulizer gas is used. A dry aerosol produced by laser ablation (LA) of biological sample and a desolvated aerosol generated by pneumatic nebulization (PN) of standard solutions are carried by two different flows of argon as carrier or nebulizer gas, respectively and introduced separately in the injector tube of a special ICP torch, through two separated apertures. Both argon flows are mixed directly in the ICP torch. External calibration via defined standard solutions before analysis of single hair was employed as calibration strategy. A correction factor, calculated using hair with known analyte concentration (measured by ICP-MS), is applied to correct the different elemental sensitivities of ICP-MS and LA-ICP-MS. Calibration curves are obtained by plotting the ratio of analyte ion M(+)/(34)S(+) ion intensities measured using LA-ICP-MS in dependence of analyte concentration in calibration solutions. Matrix-matched on-line calibration in LA-ICP-MS is carried out by ablating of human hair strands (mounted on a sticky tape in the LA chamber) using a focused laser beam in parallel with conventional nebulization of calibration solutions. Calibrations curves of Li, Na, Mg, Al, K, V, Cr, Mn, Fe, Ni, Co, Cu, Zn, Sr, Mo, Ag, Cd, I, Hg, Pb, Tl, Bi and U are presented. The linear correlation coefficients (R) of calibration curves for analytes were typically between 0.97 and 0.999. The limits of detection (LODs) of

  11. A gas-jet transport and catcher technique for on-line production of radioactive ion beams using an electron cyclotron resonance ion-source

    NASA Astrophysics Data System (ADS)

    Naik, V.; Chakrabarti, A.; Bhattacharjee, M.; Karmakar, P.; Bandyopadhyay, A.; Bhattacharjee, S.; Dechoudhury, S.; Mondal, M.; Pandey, H. K.; Lavanyakumar, D.; Mandi, T. K.; Dutta, D. P.; Kundu Roy, T.; Bhowmick, D.; Sanyal, D.; Srivastava, S. C. L.; Ray, A.; Ali, Md. S.

    2013-03-01

    Radioactive ion beams (RIB) have been produced on-line, using a gas-jet recoil transport coupled Electron Cyclotron Resonance (ECR) ion-source at the VECC-RIB facility. Radioactive atoms/molecules carried through the gas-jet were stopped in a catcher placed inside the ECR plasma chamber. A skimmer has been used to remove bulk of the carrier gas at the ECR entrance. The diffusion of atoms/molecules through the catcher has been verified off-line using stable isotopes and on-line through transmission of radioactive reaction products. Beams of 14O (71 s), 42K (12.4 h), 43K (22.2 h), and 41Ar (1.8 h) have been produced by bombarding nitrogen and argon gas targets with proton and alpha particle beams from the K130 cyclotron at VECC. Typical measured intensity of RIB at the separator focal plane is found to be a few times 103 particles per second (pps). About 3.2 × 103 pps of 1.4 MeV 14O RIB has been measured after acceleration through a radiofrequency quadrupole linac. The details of the gas-jet coupled ECR ion-source and RIB production experiments are presented along with the plans for the future.

  12. On-line double isotope dilution laser ablation inductively coupled plasma mass spectrometry for the quantitative analysis of solid materials.

    PubMed

    Fernández, Beatriz; Rodríguez-González, Pablo; García Alonso, J Ignacio; Malherbe, Julien; García-Fonseca, Sergio; Pereiro, Rosario; Sanz-Medel, Alfredo

    2014-12-01

    We report on the determination of trace elements in solid samples by the combination of on-line double isotope dilution and laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS). The proposed method requires the sequential analysis of the sample and a certified natural abundance standard by on-line IDMS using the same isotopically-enriched spike solution. In this way, the mass fraction of the analyte in the sample can be directly referred to the certified standard so the previous characterization of the spike solution is not required. To validate the procedure, Sr, Rb and Pb were determined in certified reference materials with different matrices, including silicate glasses (SRM 610, 612 and 614) and powdered samples (PACS-2, SRM 2710a, SRM 1944, SRM 2702 and SRM 2780). The analysis of powdered samples was carried out both by the preparation of pressed pellets and by lithium borate fusion. Experimental results for the analysis of powdered samples were in agreement with the certified values for all materials. Relative standard deviations in the range of 6-21% for pressed pellets and 3-21% for fused solids were obtained from n=3 independent measurements. Minimal sample preparation, data treatment and consumption of the isotopically-enriched isotopes are the main advantages of the method over previously reported approaches.

  13. On-Line Desalting of Crude Oil in the Source Region of a Fourier Transform Ion Cyclotron Resonance Mass Spectrometer

    NASA Astrophysics Data System (ADS)

    Chanthamontri, C. Ken; Stopford, Andrew P.; Snowdon, Ryan W.; Oldenburg, Thomas B. P.; Larter, Stephen R.

    2014-08-01

    The presence of dissolved metal ions in waters associated with crude oils has many negative implications for the transport, processing, and refining of petroleum. In addition, mass spectrometric analysis of sodium containing crude oil samples suffers from ionization suppression, unwanted adduct formation, and an increase in the complexity of data analysis. Here, we describe a method for the reduction/elimination of these adverse effects by modification of the source region gas-inlet system of a 12 T Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer. Several acids were examined as part of this study, with the most suitable for on-line desalting found to have both high vapor pressure and low pKa; 12.1 M HCl showed the strongest desalting effect for crude oil samples with a sodium removal index (SRI) of 88%-100% ± 7% for the NaOS compound class. In comparison, a SRI of only 38% ± 9% was observed for a H2O/toluene solution-phase extraction of Oil 1. These results clearly demonstrate the increased efficacy of pseudo-vapor phase desalting with the additional advantages that initial sample solution conditions are preserved and no sample preparation is required prior to analysis.

  14. On-line desalting of crude oil in the source region of a Fourier transform ion cyclotron resonance mass spectrometer.

    PubMed

    Chanthamontri, C Ken; Stopford, Andrew P; Snowdon, Ryan W; Oldenburg, Thomas B P; Larter, Stephen R

    2014-08-01

    The presence of dissolved metal ions in waters associated with crude oils has many negative implications for the transport, processing, and refining of petroleum. In addition, mass spectrometric analysis of sodium containing crude oil samples suffers from ionization suppression, unwanted adduct formation, and an increase in the complexity of data analysis. Here, we describe a method for the reduction/elimination of these adverse effects by modification of the source region gas-inlet system of a 12 T Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer. Several acids were examined as part of this study, with the most suitable for on-line desalting found to have both high vapor pressure and low pK(a); 12.1 M HCl showed the strongest desalting effect for crude oil samples with a sodium removal index (SRI) of 88%-100% ± 7% for the NaOS compound class. In comparison, a SRI of only 38% ± 9% was observed for a H₂O/toluene solution-phase extraction of oil 1. These results clearly demonstrate the increased efficacy of pseudo-vapor phase desalting with the additional advantages that initial sample solution conditions are preserved and no sample preparation is required prior to analysis.

  15. Laser-cooled continuous ion beams

    SciTech Connect

    Schiffer, J.P.; Hangst, J.S.; Nielsen, J.S.

    1995-08-01

    A collaboration with a group in Arhus, Denmark, using their storage ring ASTRID, brought about better understanding of ion beams cooled to very low temperatures. The longitudinal Schottky fluctuation noise signals from a cooled beam were studied. The fluctuation signals are distorted by the effects of space charge as was observed in earlier measurements at other facilities. However, the signal also exhibits previously unobserved coherent components. The ions` velocity distribution, measured by a laser fluorescence technique suggests that the coherence is due to suppression of Landau damping. The observed behavior has important implications for the eventual attainment of a crystalline ion beam in a storage ring. A significant issue is the transverse temperature of the beam -- where no direct diagnostics are available and where molecular dynamics simulations raise interesting questions about equilibrium.

  16. Calcium and lithium ion production for laser ion source

    SciTech Connect

    Okamura, M.; Palm, K.; Stifler, C.; Steski, D.; Ikeda, S.; Kumaki, M.; Kanesue, T.

    2015-08-23

    Calcium and lithium ion beams are required by NASA Space Radiation Laboratory (NSRL) at Brookhaven National Laboratory (BNL) to simulate the effects of cosmic radiation. To find out difficulties to provide such high reactive material as laser targets, the both species were experimentally tested. Plate-shaped lithium and calcium targets were fabricated to create ablation plasmas with a 6ns, 1064nm Nd:YAG laser. We found significant oxygen contamination in both the Ca and Li high-charge-state beams due to the rapid oxidation of the surfaces. A large-spot-size, low-power-density laser was then used to analyze the low-charge-state beams without scanning the targets. The low-charge-state Ca beam did not have any apparent oxygen contamination, showing the potential to clean the target entirely with a low-power beam once in the chamber. The Li target was clearly still oxidizing in the chamber after each low-power shot. To measure the rate of oxidation, we shot the low-power laser at the target repeatedly at 10sec, 30sec, 60sec, and 120sec interval lengths, showing a linear relation between the interval time and the amount of oxygen in the beam.

  17. Calcium and lithium ion production for laser ion source

    NASA Astrophysics Data System (ADS)

    Okamura, M.; Palm, K.; Stifler, C.; Steski, D.; Ikeda, S.; Kumaki, M.; Kanesue, T.

    2016-02-01

    Calcium and lithium ion beams are required by NASA Space Radiation Laboratory at Brookhaven National Laboratory to simulate the effects of cosmic radiation. To identify the difficulties in providing such highly reactive materials as laser targets, both species were experimentally tested. Plate shaped lithium and calcium targets were fabricated to create ablation plasmas with a 6 ns 1064 nm neodymium-doped yttrium aluminum garnet laser. We found significant oxygen contamination in both the Ca and Li high charge state beams due to the rapid oxidation of the surfaces. A large spot size, low power density laser was used to create low charge state beams without scanning the targets. The low charge state Ca beam did not have any apparent oxygen contamination, showing the potential to clean the target entirely of oxide with a low power beam once in the chamber. The Li target was clearly still oxidizing in the chamber after each low power shot. To measure the rate of oxidation, we shot the low power laser at the target repeatedly at 10 s, 30 s, 60 s, and 120 s interval lengths, showing a linear relation between the interval time and the amount of oxygen in the beam.

  18. Calcium and lithium ion production for laser ion source.

    PubMed

    Okamura, M; Palm, K; Stifler, C; Steski, D; Ikeda, S; Kumaki, M; Kanesue, T

    2016-02-01

    Calcium and lithium ion beams are required by NASA Space Radiation Laboratory at Brookhaven National Laboratory to simulate the effects of cosmic radiation. To identify the difficulties in providing such highly reactive materials as laser targets, both species were experimentally tested. Plate shaped lithium and calcium targets were fabricated to create ablation plasmas with a 6 ns 1064 nm neodymium-doped yttrium aluminum garnet laser. We found significant oxygen contamination in both the Ca and Li high charge state beams due to the rapid oxidation of the surfaces. A large spot size, low power density laser was used to create low charge state beams without scanning the targets. The low charge state Ca beam did not have any apparent oxygen contamination, showing the potential to clean the target entirely of oxide with a low power beam once in the chamber. The Li target was clearly still oxidizing in the chamber after each low power shot. To measure the rate of oxidation, we shot the low power laser at the target repeatedly at 10 s, 30 s, 60 s, and 120 s interval lengths, showing a linear relation between the interval time and the amount of oxygen in the beam. PMID:26931962

  19. Theory of the ion-channel laser

    SciTech Connect

    Whittum, D.H.

    1990-09-01

    A relativistic electron beam propagating through a plasma in the ion-focussed regime exhibits an electromagnetic instability with peak growth rate near a resonant frequency {omega}{approximately}2 {gamma}{sup 2} {omega}{beta}, where {gamma} is the Lorentz factor and {omega}{beta} is the betatron frequency. The physical basis for this instability is that an ensemble of relativistic simple harmonic oscillators, weakly driven by an electromagnetic wave, will lose energy to the wave through axial bunching. This bunching'' corresponds to the development of an rf component in the beam current, and a coherent centroid oscillation. The subject of this thesis is the theory of a laser capitalizing on this electromagnetic instability. A historical perspective is offered. The basic features of relativistic electron beam propagation in the ion-focussed regime are reviewed. The ion-channel laser (ICL) instability is explored theoretically through an eikonal formalism, analgous to the KMR'' formalism for the free-electron laser (FEL). The dispersion relation is derived, and the dependence of growth rate on three key parameters is explored. Finite temperature effects are assessed. From this work it is found that the typical gain length for amplification is longer than the Rayleigh length and we go on to consider three mechanisms which will tend to guide waveguide. First, we consider the effect of the ion channel as a dielectric waveguide. We consider next the use of a conducting waveguide, appropriate for a microwave amplifier. Finally, we examine a form of optical guiding'' analgous to that found in the FEL. The eikonal formalism is used to model numerically the instability through and beyond saturation. Results are compared with the numerical simulation of the full equations of motion, and with the analytic scalings. The analytical requirement on detuning spread is confirmed.

  20. In-Source Laser Spectroscopy with the Laser Ion Source and Trap: First Direct Study of the Ground-State Properties of Po,219217

    NASA Astrophysics Data System (ADS)

    Fink, D. A.; Cocolios, T. E.; Andreyev, A. N.; Antalic, S.; Barzakh, A. E.; Bastin, B.; Fedorov, D. V.; Fedosseev, V. N.; Flanagan, K. T.; Ghys, L.; Gottberg, A.; Huyse, M.; Imai, N.; Kron, T.; Lecesne, N.; Lynch, K. M.; Marsh, B. A.; Pauwels, D.; Rapisarda, E.; Richter, S. D.; Rossel, R. E.; Rothe, S.; Seliverstov, M. D.; Sjödin, A. M.; Van Beveren, C.; Van Duppen, P.; Wendt, K. D. A.

    2015-01-01

    A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. It offers two modes of operation, either as an ion guide, which performs similarly to the standard ISOLDE resonance ionization laser ion source (RILIS), or as a more selective ion source, where surface-ionized ions from the hot ion-source cavity are repelled by an electrode, while laser ionization is done within a radio-frequency quadrupole ion guide. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of 217Po for the first time. Nuclear decay spectroscopy of 219Po is performed for the first time, revealing its half-life, α -to-β -decay branching ratio, and α -particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes.

  1. Directional Laser-Driven Ion Acceleration from Microspheres

    SciTech Connect

    Sokollik, T.; Schnuerer, M.; Steinke, S.; Nickles, P. V.; Sandner, W.; Amin, M.; Toncian, T.; Willi, O.; Andreev, A. A.

    2009-09-25

    Laser-driven ion acceleration is capable of generating ion beams of MeV energy exhibiting unique attributes such as ultralow emittance. Research is still focusing on fundamental laser-target interactions to control further beam attributes. In this Letter we present the observation of directional ion acceleration of irradiated spherical targets through proton imaging. This feature, together with an earlier observed quasimonoenergetic proton burst makes spherical targets extremely attractive candidates for high quality, high repetition rate sources of laser accelerated particles.

  2. Laser ion acceleration toward future ion beam cancer therapy - Numerical simulation study -

    PubMed Central

    Kawata, Shigeo; Izumiyama, Takeshi; Nagashima, Toshihiro; Takano, Masahiro; Barada, Daisuke; Kong, Qing; Gu, Yan Jun; Wang, Ping Xiao; Ma, Yan Yun; Wang, Wei Min

    2013-01-01

    Background: Ion beam has been used in cancer treatment, and has a unique preferable feature to deposit its main energy inside a human body so that cancer cell could be killed by the ion beam. However, conventional ion accelerator tends to be huge in its size and its cost. In this paper a future intense-laser ion accelerator is proposed to make the ion accelerator compact. Subjects and methods: An intense femtosecond pulsed laser was employed to accelerate ions. The issues in the laser ion accelerator include the energy efficiency from the laser to the ions, the ion beam collimation, the ion energy spectrum control, the ion beam bunching and the ion particle energy control. In the study particle computer simulations were performed to solve the issues, and each component was designed to control the ion beam quality. Results: When an intense laser illuminates a target, electrons in the target are accelerated and leave from the target; temporarily a strong electric field is formed between the high-energy electrons and the target ions, and the target ions are accelerated. The energy efficiency from the laser to ions was improved by using a solid target with a fine sub-wavelength structure or by a near-critical density gas plasma. The ion beam collimation was realized by holes behind the solid target. The control of the ion energy spectrum and the ion particle energy, and the ion beam bunching were successfully realized by a multi-stage laser-target interaction. Conclusions: The present study proposed a novel concept for a future compact laser ion accelerator, based on each component study required to control the ion beam quality and parameters. PMID:24155555

  3. A new lithium-ion battery internal temperature on-line estimate method based on electrochemical impedance spectroscopy measurement

    NASA Astrophysics Data System (ADS)

    Zhu, J. G.; Sun, Z. C.; Wei, X. Z.; Dai, H. F.

    2015-01-01

    The power battery thermal management problem in EV (electric vehicle) and HEV (hybrid electric vehicle) has been widely discussed, and EIS (electrochemical impedance spectroscopy) is an effective experimental method to test and estimate the status of the battery. Firstly, an electrochemical-based impedance matrix analysis for lithium-ion battery is developed to describe the impedance response of electrochemical impedance spectroscopy. Then a method, based on electrochemical impedance spectroscopy measurement, has been proposed to estimate the internal temperature of power lithium-ion battery by analyzing the phase shift and magnitude of impedance at different ambient temperatures. Respectively, the SoC (state of charge) and temperature have different effects on the impedance characteristics of battery at various frequency ranges in the electrochemical impedance spectroscopy experimental study. Also the impedance spectrum affected by SoH (state of health) is discussed in the paper preliminary. Therefore, the excitation frequency selected to estimate the inner temperature is in the frequency range which is significantly influenced by temperature without the SoC and SoH. The intrinsic relationship between the phase shift and temperature is established under the chosen excitation frequency. And the magnitude of impedance related to temperature is studied in the paper. In practical applications, through obtaining the phase shift and magnitude of impedance, the inner temperature estimation could be achieved. Then the verification experiments are conduced to validate the estimate method. Finally, an estimate strategy and an on-line estimation system implementation scheme utilizing battery management system are presented to describe the engineering value.

  4. Origin of 'energetic' ions from laser-produced plasmas.

    NASA Technical Reports Server (NTRS)

    Ehler, W.; Linlor, W. I.

    1973-01-01

    A fast-ion current peak, measured with an ion collector placed in the path of an expanding laser-produced plasma, was identified as carbon, nitrogen, and oxygen contaminants which originated from a tungsten target surface.

  5. Determination of ammonium ion by fluorometry or spectrophotometry after on-line derivatization with o-phthalaldehyde

    NASA Technical Reports Server (NTRS)

    Goyal, S. S.; Rains, D. W.; Huffaker, R. C.

    1988-01-01

    A fast, sensitive, simple, and highly reproducible method for routine assay of ammonium ion (NH4+) was developed by using HPLC equipment. The method is based on the reaction of NH4+ with o-phthalaldehyde (OPA) in the presence of 2-mercaptoethanol. After an on-line derivatization, the resulting NH4(+)-OPA product was quantified by using fluorometric or spectrophotometric detection. For fluorometric detection, the excitation and emission wavelengths were 410 and 470 nm, respectively. The spectrophotometric detection was made by measuring absorbance at 410 nm. Results on the effects of OPA-reagent composition and pH, reaction temperature, sample matrix, and linearity of the assay are presented. Even though it took about 2 min from the time of sample injection to the appearance of sample peak, sample injections could be overlapped at an interval of about 1 min. Thus, the actual time needed for analysis was about 1 min per assay. The method can be used in a fully automated mode by using an autosampler injector.

  6. Post-acceleration of laser-induced ion beams

    NASA Astrophysics Data System (ADS)

    Nassisi, V.; Delle Side, D.

    2015-04-01

    A complete review of the essential and recent developments in the field of post-acceleration of laser-induced ion beams is presented. After a brief introduction to the physics of low-intensity nanosecond laser-matter interaction, the details of ions extraction and acceleration are critically analyzed and the key parameters to obtain good-quality ion beams are illustrated. A description of the most common ion beam diagnosis system is given, together with the associated analytical techniques.

  7. Diagnostics for studies of novel laser ion acceleration mechanisms

    SciTech Connect

    Senje, Lovisa; Aurand, Bastian; Wahlström, Claes-Göran; Yeung, Mark; Kuschel, Stephan; Rödel, Christian; Wagner, Florian; Roth, Markus; Li, Kun; Neumayer, Paul; Dromey, Brendan; Jung, Daniel; Bagnoud, Vincent; Zepf, Matthew; Kuehl, Thomas

    2014-11-15

    Diagnostic for investigating and distinguishing different laser ion acceleration mechanisms has been developed and successfully tested. An ion separation wide angle spectrometer can simultaneously investigate three important aspects of the laser plasma interaction: (1) acquire angularly resolved energy spectra for two ion species, (2) obtain ion energy spectra for multiple species, separated according to their charge to mass ratio, along selected axes, and (3) collect laser radiation reflected from and transmitted through the target and propagating in the same direction as the ion beam. Thus, the presented diagnostic constitutes a highly adaptable tool for accurately studying novel acceleration mechanisms in terms of their angular energy distribution, conversion efficiency, and plasma density evolution.

  8. Diagnostics for studies of novel laser ion acceleration mechanisms.

    PubMed

    Senje, Lovisa; Yeung, Mark; Aurand, Bastian; Kuschel, Stephan; Rödel, Christian; Wagner, Florian; Li, Kun; Dromey, Brendan; Bagnoud, Vincent; Neumayer, Paul; Roth, Markus; Wahlström, Claes-Göran; Zepf, Matthew; Kuehl, Thomas; Jung, Daniel

    2014-11-01

    Diagnostic for investigating and distinguishing different laser ion acceleration mechanisms has been developed and successfully tested. An ion separation wide angle spectrometer can simultaneously investigate three important aspects of the laser plasma interaction: (1) acquire angularly resolved energy spectra for two ion species, (2) obtain ion energy spectra for multiple species, separated according to their charge to mass ratio, along selected axes, and (3) collect laser radiation reflected from and transmitted through the target and propagating in the same direction as the ion beam. Thus, the presented diagnostic constitutes a highly adaptable tool for accurately studying novel acceleration mechanisms in terms of their angular energy distribution, conversion efficiency, and plasma density evolution.

  9. Sympathetic cooling of laser-produced doubly charged ions in a few-ion crystal

    SciTech Connect

    Kwapien, T.; Eichmann, U.; Sandner, W.

    2007-06-15

    We present experimental results in which single Ca{sup +} ions in a chain of laser cooled Ca{sup +} ions are further ionized by means of an intense short pulse laser. The ions are trapped in a linear Paul trap, which is instantaneously loaded by ions from a laser-produced ablation plasma. Due to sympathetic cooling the doubly charged ions are held in place. We study and characterize linear few-ion crystals with mixed charges by applying a radio frequency field, which excites the center of mass (c.m.) and breathing modes of different configurations. From the position shift of laser cooled ions initiated through the higher charge state we can deduce the charge of the nonfluorescing ion. This information might be used as an intensity probe for high intensity lasers.

  10. Laser-cooled bunched ion beam

    SciTech Connect

    Schiffer, J.P.; Hangst, J.S.; Nielsen, J.S.

    1995-08-01

    In collaboration with the Arhus group, the laser cooling of a beam bunched by an rf electrode was investigated at the ASTRID storage ring. A single laser is used for unidirectional cooling, since the longitudinal velocity of the beam will undergo {open_quotes}synchrotron oscillations{close_quotes} and the ions are trapped in velocity space. As the cooling proceeds the velocity spread of the beam, as well as the bunch length is measured. The bunch length decreases to the point where it is limited only by the Coulomb repulsion between ions. The measured length is slightly (20-30%) smaller than the calculated limit for a cold beam. This may be the accuracy of the measurement, or may indicate that the beam still has a large transverse temperature so that the longitudinal repulsion is less than would be expected from an absolutely cold beam. Simulations suggest that the coupling between transverse and longitudinal degrees of freedom is strong -- but this issue will have to be resolved by further measurements.

  11. A novel Laser Ion Mobility Spectrometer

    NASA Astrophysics Data System (ADS)

    Göbel, J.; Kessler, M.; Langmeier, A.

    2009-05-01

    IMS is a well know technology within the range of security based applications. Its main advantages lie in the simplicity of measurement, along with a fast and sensitive detection method. Contemporary technology often fails due to interference substances, in conjunction with saturation effects and a low dynamic detection range. High throughput facilities, such as airports, require the analysis of many samples at low detection limits within a very short timeframe. High detection reliability is a requirement for safe and secure operation. In our present work we developed a laser based ion-mobility-sensor which shows several advantages over known IMS sensor technology. The goal of our research was to increase the sensitivity compared to the range of 63Ni based instruments. This was achieved with an optimised geometric drift tube design and a pulsed UV laser system at an efficient intensity. In this intensity range multi-photon ionisation is possible, which leads to higher selectivity in the ion-formation process itself. After high speed capturing of detection samples, a custom designed pattern recognition software toolbox provides reliable auto-detection capability with a learning algorithm and a graphical user interface.

  12. Development of laser noninvasive on-line diagnostics of oncological diseases based on the absorption method in the 4860-4880 cm-1 spectral range

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Shnyrev, S. L.; Kondrashov, A. A.

    2016-07-01

    A novel method for noninvasive on-line diagnostics of gastrointestinal oncological diseases using a diode laser in the 4860-4880 cm-1 frequency range is proposed. The method is based on measuring the concentration of 13C during expiration. The accuracy of the method allows performing early diagnostics of diseases.

  13. Applying the diode laser spectroscopy method for high sensitivity on-line control of 13C contained in the gaseous mixture with 12C

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Kondrashov, A. A.; Shnyrev, S. L.

    2016-06-01

    This letter details the development of an on-line control method for carbon dioxide molecules of various isotopes contained in gaseous media on the basis of a tunable diode laser operating in the 4860-4880 cm-1 range. It shows that the sensitivity of 13C registering may amount to ~1012 cm-3.

  14. Applying the diode laser spectroscopy method for high sensitivity on-line control of 13С contained in the gaseous mixture with 12С

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Kondrashov, A. A.; Shnyrev, S. L.

    2016-06-01

    This letter details the development of an on-line control method for carbon dioxide molecules of various isotopes contained in gaseous media on the basis of a tunable diode laser operating in the 4860–4880 cm‑1 range. It shows that the sensitivity of 13С registering may amount to ~1012 cm‑3.

  15. Development of laser noninvasive on-line diagnostics of oncological diseases based on the absorption method in the 4860–4880 cm‑1 spectral range

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Shnyrev, S. L.; Kondrashov, A. A.

    2016-07-01

    A novel method for noninvasive on-line diagnostics of gastrointestinal oncological diseases using a diode laser in the 4860–4880 cm‑1 frequency range is proposed. The method is based on measuring the concentration of 13С during expiration. The accuracy of the method allows performing early diagnostics of diseases.

  16. On-line detection of heavy metals and brominated flame retardants in technical polymers with laser-induced breakdown spectrometry.

    PubMed

    Stepputat, Michael; Noll, Reinhard

    2003-10-20

    The use of laser-induced breakdown spectrometry (LIBS) for the analysis of heavy metals and brominated flame retardants in end-of-life waste electric and electronic equipment (EOL-WEEE) pieces is investigated. Single- and double-pulse plasma excitation as well as the influence of detection parameters is studied to yield a parameter field with improved sensitivity and limits of detection. A LIBS analyzer was set up as an on-line measuring unit to detect heavy metals and brominated flame retardants in moving EOL-WEEE pieces in an automatic sorting line. An autofocusing unit with an adjustment range of 50 mm was incorporated to permit measurements of objects that pass by a LIBS analyzer with their surfaces at various distances from it. Tests with EOL-WEEE monitor housings on the conveyor belt of a pilot sorting system successfully demonstrated the capability of the LIBS analyzer to quantify the concentration of hazardous elements in real waste EOL-WEEE pieces. PMID:14594087

  17. On-line detection of heavy metals and brominated flame retardants in technical polymers with laser-induced breakdown spectrometry

    NASA Astrophysics Data System (ADS)

    Stepputat, Michael; Noll, Reinhard

    2003-10-01

    The use of laser-induced breakdown spectrometry (LIBS) for the analysis of heavy metals and brominated flame retardants in end-of-life waste electric and electronic equipment (EOL-WEEE) pieces is investigated. Single- and double-pulse plasma excitation as well as the influence of detection parameters is studied to yield a parameter field with improved sensitivity and limits of detection. A LIBS analyzer was set up as an on-line measuring unit to detect heavy metals and brominated flame retardants in moving EOL-WEEE pieces in an automatic sorting line. An autofocusing unit with an adjustment range of 50 mm was incorporated to permit measurements of objects that pass by a LIBS analyzer with their surfaces at various distances from it. Tests with EOL-WEEE monitor housings on the conveyor belt of a pilot sorting system successfully demonstrated the capability of the LIBS analyzer to quantify the concentration of hazardous elements in real waste EOL-WEEE pieces.

  18. Interaction of plasmas in laser ion source with double laser system

    SciTech Connect

    Fuwa, Y.; Ikeda, S.; Kumaki, M.; Sekine, M.; Cinquegrani, D.; Romanelli, M.; Kanesue, T.; Okamura, M.; Iwashita, Y.

    2014-02-15

    Multiple laser shots could be used to elongate an ion beam pulse width or to intensify beam current from laser ion sources. In order to confirm the feasibility of the multiple shot scheme, we investigated the properties of plasmas produced by double laser shots. We found that when the interval of the laser shots is shorter than 10 μs, the ion current profile had a prominent peak, which is not observed in single laser experiments. The height of this peak was up to five times larger than that of single laser experiment.

  19. Laser Induced Fluorescence of the Iodine Ion

    NASA Astrophysics Data System (ADS)

    Hargus, William

    2014-10-01

    Iodine (I2) has been considered as a potential electrostatic spacecraft thruster propellant for approximately 2 decades, but has only recently been demonstrated. Energy conversion efficiency appears to be on par with xenon without thruster modification. Intriguingly, performance appears to exceed xenon at high acceleration potentials. As part of a continuing program for the development of non-intrusive plasma diagnostics for advanced plasma spacecraft propulsion, we have identified the I II 5d5D4 o state as metastable, and therefore containing a reservoir of excited state ions suitable for laser probing. The 5d5D4 o - 6p5P3 transition at 695.878 nm is convenient for diode laser excitation with the 5s5S2 o - 6p5P3 transition at 516.12 nm as an ideal candidate for non-resonant fluorescence collection. We have constructed a Penning type iodine microwave discharge lamp optimized for I II production for table-top measurements. This work demonstrates I II laser-induced fluorescence in a representative iodine discharge and will validate our previous theoretical work based on the limited available historical I II spectral data.

  20. New laser setup for the selective isotope production and investigation in a laser ion source at the IRIS (Investigation of Radioactive Isotopes on Synchrocyclotron) facility

    SciTech Connect

    Barzakh, A. E.; Fedorov, D. V.; Ivanov, V. S.; Molkanov, P. L.; Panteleev, V. N.; Volkov, Yu. M.

    2012-02-15

    New laser installation for the resonance ionization spectroscopy in a laser ion source and for rare isotope production has been recently put into operation at the IRIS (Investigation of Radioactive Isotopes on Synchrocyclotron) facility (Petersburg Nuclear Physics Institute, Gatchina). This is a significant improvement of a previous target-laser ion source device of the IRIS mass-separator, working on-line with 1 GeV proton beam of PNPI (Petersburg Nuclear Physics Institute) synchrocyclotron. It makes possible for us to get the isobarically clean radioactive isotope beams of a great number of chemical elements. New laser setup provides the two- or three-resonance step ionization in the range of wavelength of 265-850 nm. The first results obtained at the laser setup for Tl isotopes are presented.

  1. Gravitational waves generated by laser accelerated relativistic ions

    NASA Astrophysics Data System (ADS)

    Gelfer, Evgeny G.; Kadlecová, Hedvika; Klimo, Ondřej; Weber, Stefan; Korn, Georg

    2016-09-01

    The generation of gravitational waves by laser accelerated relativistic ions is investigated. The piston and light sail models of laser plasma acceleration are considered, and analytical expressions for space-time metric perturbation are derived. For both models, the dependence of gravitational wave amplitude on the laser and plasma parameters as well as gravitational wave spectrum and angular distribution is examined.

  2. Magnetic plasma confinement for laser ion source.

    PubMed

    Okamura, M; Adeyemi, A; Kanesue, T; Tamura, J; Kondo, K; Dabrowski, R

    2010-02-01

    A laser ion source (LIS) can easily provide a high current beam. However, it has been difficult to obtain a longer beam pulse while keeping a high current. On occasion, longer beam pulses are required by certain applications. For example, more than 10 micros of beam pulse is required for injecting highly charged beams to a large sized synchrotron. To extend beam pulse width, a solenoid field was applied at the drift space of the LIS at Brookhaven National Laboratory. The solenoid field suppressed the diverging angle of the expanding plasma and the beam pulse was widened. Also, it was observed that the plasma state was conserved after passing through a few hundred gauss of the 480 mm length solenoid field.

  3. Improved Analytical Performance of Negative 63Ni Ion Mobility Spectrometry for On-line Measurement of Propofol Using Dichloromethane as Dopant

    NASA Astrophysics Data System (ADS)

    Zhou, Qinghua; Hua, Lei; Wang, Changsong; Li, Enyou; Li, Haiyang

    2015-01-01

    On-line monitoring of propofol in exhaled air is a potential way to evaluate the anaesthesia depth for patients during surgery. In this study, a negative 63Ni ionization high resolution ion mobility spectrometer with Bradbury-Nielsen-Gate-Grid structure was built to measure propofol with reactant ions Cl-(H2O) n using dichloromethane as dopant. Instead of forming three propofol ions (M - H)-, M · O2 -, and (M2 - H)- with reactant ions O2 -(H2O) n , only product ion M · Cl- was produced when introducing dichloromethane gas. The peak-to-peak resolution ( R p-p) between reactant ions Cl-(H2O) n and product ion M · Cl- was 17.4, which was 1.6 times larger than that between O2 -(H2O) n and product ion. Furthermore, the linear response range using reactant ions Cl-(H2O) n was 3.5 times wider than that obtained with reactant ions O2 -(H2O) n .

  4. Analysis of Ion Currents Generated with a Pulsed Laser

    SciTech Connect

    Krasa, J.; Jungwirth, K.; Krousky, E.; Laska, L.; Pfeifer, M.; Rohlena, K.; Velyhan, A.; Ullschmied, J.

    2008-03-19

    A deconvolution analysis of ion currents, which is based on the use of shifted Maxwell-Boltzmann velocity distribution, is applied to determine the temperatures and the centre-of-mass velocities of ions emitted from polyethylene and Cu targets irradiated by pulsed laser beams. This analysis can render important details in establishing the mechanisms responsible for the ion emission.

  5. Hot-cavity studies for the Resonance Ionization Laser Ion Source

    NASA Astrophysics Data System (ADS)

    Henares, J. L.; Lecesne, N.; Hijazi, L.; Bastin, B.; Kron, T.; Lassen, J.; Le Blanc, F.; Leroy, R.; Osmond, B.; Raeder, S.; Schneider, F.; Wendt, K.

    2016-09-01

    The Resonance Ionization Laser Ion Source (RILIS) has emerged as an important technique in many Radioactive Ion Beam (RIB) facilities for its reliability, and ability to ionize target elements efficiently and element selectively. GISELE is an off-line RILIS test bench to study the implementation of an on-line laser ion source at the GANIL separator facility. The aim of this project is to determine the best technical solution which combines high selectivity and ionization efficiency with small ion beam emittance and stable long term operation. The ion source geometry was tested in several configurations in order to find a solution with optimal ionization efficiency and beam emittance. Furthermore, a low work function material was tested to reduce the contaminants and molecular sidebands generated inside the ion source. First results with ZrC ionizer tubes will be presented. Furthermore, a method to measure the energy distribution of the ion beam as a function of the time of flight will be discussed.

  6. Pulsed UV laser induced desorption of ions from aluminum

    NASA Astrophysics Data System (ADS)

    Taylor, David Paul; Helvajian, Henry

    2000-04-01

    A study of pulsed UV laser induced desorption (LID) has been performed on an Al(111) sample. The positive ion desorption was investigated at low laser fluence, in a regime in which the ion yield exhibits a highly non-linear dependence on the laser fluence. The peak of the kinetic energy distribution of the desorbed ions has been measured to be about 15 eV. This result is consistent with the conjecture that the ion departing the metal surface can acquire a kinetic energy kick from a process associated with plasmon annihilation. The Al + ion kinetic energy peak is asymmetric and about 3 eV full-width at half-maximum (FWHM). This experiment indicates that plasmon excitation can play a significant role in laser stimulated desorption induced by electronic transitions (DIET).

  7. Production of negative osmium ions by laser desorption and ionization.

    PubMed

    Rodríguez, D; Sonnenschein, V; Blaum, K; Block, M; Kluge, H-J; Lallena, A M; Raeder, S; Wendt, K

    2010-01-01

    The interest to produce negative osmium ions is manifold in the realm of high-accuracy ion trap experiments: high-resolution nearly Doppler-free laser spectroscopy, antihydrogen formation in its ground state, and contributions to neutrino mass spectrometry. Production of these ions is generally accomplished by sputtering an Os sample with Cs(+) ions at tens of keV. Though this is a well-established method commonly used at accelerators, these kind of sources are quite demanding and tricky to operate. Therefore, the development of a more straightforward and cost effective production scheme will be of benefit for ion trap and other experiments. Such a scheme makes use of desorption and ionization with pulsed lasers and identification of the ions by time-of-flight mass spectrometry. First investigations of negative osmium ion production using a pulsed laser for desorption and ionization and a commercial matrix-assisted laser desorption/ionization time-of-flight system for identification has demonstrated the suitability of this technique. More than 10(3) negative osmium ions per shot were registered after bombarding pure osmium powder with a 5 ns pulse width Nd:yttrium aluminum garnet laser. The limitation in the ion number was imposed by the detection limit of the microchannel plate detector.

  8. On-line molecular iodine isotopologue detection in gaseous media during spent nuclear fuel reprocessing using a laser-induced fluorescence method

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Shnyrev, S. L.

    2015-06-01

    The paper reports on on-line measurement of the {}129{{\\text{I}}2}, 127I129I, and {}127{{\\text{I}}2} concentrations during spent nuclear fuel (SNF) reprocessing using a laser-induced fluorescence method. A He-Ne laser (632.8 nm) was used as a fluorescence excitation source. The detection limits obtained for molecular iodine isotopologue concentrations demonstrate the possibility of using this method for iodine control both in gaseous technological media generated during SNF reprocessing and after passing through the gas purification system (in atmosphere emission).

  9. Influence of the gaseous mixture composition on accuracy of molecular iodine on-line detection by laser-induced fluorescence method

    NASA Astrophysics Data System (ADS)

    Kireev, S. V.; Shnyrev, S. L.

    2016-07-01

    This paper informs on research into the influence of the composition of gaseous mixtures analyzed on the accuracy of on-line molecular iodine detection by laser-induced fluorescence in various gaseous media—in atmospheric air and in technological mixtures formed during reprocessing of spent nuclear fuel. The paper shows that by considering the composition of buffer media and parts of its components, the accuracy of iodine content measurement may be increased in several times.

  10. On-line selective enrichment and ion-pair reaction for structural determination of sulfated glycopeptides by capillary electrophoresis-mass spectrometry.

    PubMed

    Imami, Koshi; Ishihama, Yasushi; Terabe, Shigeru

    2008-06-20

    We describe a new capillary electrophoresis-mass spectrometry (CE-MS)-based technique for analyzing sulfated glycopeptides. The proposed method performs selective enrichment of sulfated glycopeptides from a complex mixture of peptides based on field-enhanced sample injection and ion-pair reaction with a basic ion-pair reagent (Lys-Lys-Lys; KKK) at the exit end of a capillary in a single analysis, which permits successful fragmentation of sulfated glycopeptides in positive-ion mode at the MS/MS stage for comprehensive structural analysis. In this study, the method was verified using a model sulfated monosaccharide, N-acetyl-d-galactosamine 4-sulfate (GalNAc 4S). As an example of an application of this method, sulfated glycopeptides were selectively enriched from the enzymatic digest of thyroid stimulating hormone, affording approximately 500-fold sensitivity enhancement, and structural information was successfully obtained via on-line ion-pair complexation reaction.

  11. Intense ion beams accelerated by ultra-intense laser pulses

    NASA Astrophysics Data System (ADS)

    Roth, Markus; Cowan, T. E.; Gauthier, J. C.; Vehn, J. Meyer-Ter; Allen, M.; Audebert, P.; Blazevic, A.; Fuchs, J.; Geissel, M.; Hegelich, M.; Karsch, S.; Pukhov, A.; Schlegel, T.

    2002-04-01

    The discovery of intense ion beams off solid targets irradiated by ultra-intense laser pulses has become the subject of extensive international interest. These highly collimated, energetic beams of protons and heavy ions are strongly depending on the laser parameters as well as on the properties of the irradiated targets. Therefore we have studied the influence of the target conditions on laser-accelerated ion beams generated by multi-terawatt lasers. The experiments were performed using the 100 TW laser facility at Laboratoire pour l'Utilisation des Laser Intense (LULI). The targets were irradiated by pulses up to 5×1019 W/cm2 (~300 fs,λ=1.05 μm) at normal incidence. A strong dependence on the surface conditions, conductivity, shape and purity was observed. The plasma density on the front and rear surface was determined by laser interferometry. We characterized the ion beam by means of magnetic spectrometers, radiochromic film, nuclear activation and Thompson parabolas. The strong dependence of the ion beam acceleration on the conditions on the target back surface was confirmed in agreement with predictions based on the target normal sheath acceleration (TNSA) mechanism. Finally shaping of the ion beam has been demonstrated by the appropriate tailoring of the target. .

  12. Measurement of ion beam from laser ion source for RHIC EBIS.

    SciTech Connect

    Kanesue,T.; Tamura, J.; Okamura, M.

    2008-06-23

    Laser ion source (LIS) is a candidate of the primary ion source for the RHIC EBIS. LIS will provide intense charge state 1+ ions to the EBIS for further ionization. We measured plasma properties of a variety of atomic species from C to Au using the second harmonics of Nd:YAG laser (532 nm wave length, up to 0.5 J/6 ns). Since properties of laser produced plasma is different from different species, laser power density for singly charged ion production should be verified experimentally for each atomic species. After plasma analysis experiments, Au ions was extracted from plasma and emittance of the ion beam was measured using a pepper pot type emittance monitor.

  13. Intense ion beams accelerated by relativistic laser plasmas

    NASA Astrophysics Data System (ADS)

    Roth, Markus; Cowan, Thomas E.; Gauthier, Jean-Claude J.; Allen, Matthew; Audebert, Patrick; Blazevic, Abel; Fuchs, Julien; Geissel, Matthias; Hegelich, Manuel; Karsch, S.; Meyer-ter-Vehn, Jurgen; Pukhov, Alexander; Schlegel, Theodor

    2001-12-01

    We have studied the influence of the target properties on laser-accelerated proton and ion beams generated by the LULI multi-terawatt laser. A strong dependence of the ion emission on the surface conditions, conductivity, shape and material of the thin foil targets were observed. We have performed a full characterization of the ion beam using magnetic spectrometers, Thompson parabolas, radiochromic film and nuclear activation techniques. The strong dependence of the ion beam acceleration on the conditions on the target back surface was found in agreement with theoretical predictions based on the target normal sheath acceleration (TNSA) mechanism. Proton kinetic energies up to 25 MeV have been observed.

  14. New method of beam bunching in free-ion lasers

    SciTech Connect

    Bessonov, E.G.

    1995-12-31

    An effective ion beam bunching method is suggested. This method is based on a selective interaction of line spectrum laser light (e.g. axial mode structure light) with non-fully stripped ion beam cooled in a storage rings, arranging the ion beam in layers in radial direction of an energy-longitudinal coordinate plane and following rotation of the beam at the right angle after switching on the RF cavity or undulator grouper/buncher. Laser cooling of the ion beam can be used at this position after switching off the resonator to decrease the energy spread caused by accelerating field of the resonator. A relativistic multilayer ion mirror will be produced this way. Both monochromatic laser beams and intermediate monochromaticity and bandwidth light sources of spontaneous incoherent radiation can be used for production of hard and high power electromagnetic radiation by reflection from this mirror. The reflectivity of the mirror is rather high because of the cross-section of the backward Rayleigh scattering of photon light by non-fully stripped relativistic ions ({approximately}{lambda}{sup 2}) is much greater ({approximately} 10{divided_by}15 orders) then Thompson one ({approximately} r{sub e}{sup 2}). This position is valid even in the case of non-monochromatic laser light ({Delta}{omega}/{omega} {approximately} 10{sup -4}). Ion cooling both in longitudinal plane and three-dimensional radiation ion cooling had been proposed based on this observation. The using of these cooling techniques will permit to store high current and low emittance relativistic ion beams in storage rings. The bunched ion beam can be used in ordinary Free-Ion Lasers as well. After bunching the ion beam can be extracted from the storage ring in this case. Storage rings with zero momentum compaction function will permit to keep bunching of the ion beam for a long time.

  15. Generation of elliptically polarized nitrogen ion laser fields using two-color femtosecond laser pulses

    PubMed Central

    Li, Ziting; Zeng, Bin; Chu, Wei; Xie, Hongqiang; Yao, Jinping; Li, Guihua; Qiao, Lingling; Wang, Zhanshan; Cheng, Ya

    2016-01-01

    We experimentally investigate generation of nitrogen molecular ion () lasers with two femtosecond laser pulses at different wavelengths. The first pulse serves as the pump which ionizes the nitrogen molecules and excites the molecular ions to excited electronic states. The second pulse serves as the probe which leads to stimulated emission from the excited molecular ions. We observe that changing the angle between the polarization directions of the two pulses gives rise to elliptically polarized laser fields, which is interpreted as a result of strong birefringence of the gain medium near the wavelengths of the laser. PMID:26888182

  16. Generation of elliptically polarized nitrogen ion laser fields using two-color femtosecond laser pulses.

    PubMed

    Li, Ziting; Zeng, Bin; Chu, Wei; Xie, Hongqiang; Yao, Jinping; Li, Guihua; Qiao, Lingling; Wang, Zhanshan; Cheng, Ya

    2016-02-18

    We experimentally investigate generation of nitrogen molecular ion (N2+) lasers with two femtosecond laser pulses at different wavelengths. The first pulse serves as the pump which ionizes the nitrogen molecules and excites the molecular ions to excited electronic states. The second pulse serves as the probe which leads to stimulated emission from the excited molecular ions. We observe that changing the angle between the polarization directions of the two pulses gives rise to elliptically polarized N2+ laser fields, which is interpreted as a result of strong birefringence of the gain medium near the wavelengths of the N2+ laser.

  17. Generation of elliptically polarized nitrogen ion laser fields using two-color femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Li, Ziting; Zeng, Bin; Chu, Wei; Xie, Hongqiang; Yao, Jinping; Li, Guihua; Qiao, Lingling; Wang, Zhanshan; Cheng, Ya

    2016-02-01

    We experimentally investigate generation of nitrogen molecular ion () lasers with two femtosecond laser pulses at different wavelengths. The first pulse serves as the pump which ionizes the nitrogen molecules and excites the molecular ions to excited electronic states. The second pulse serves as the probe which leads to stimulated emission from the excited molecular ions. We observe that changing the angle between the polarization directions of the two pulses gives rise to elliptically polarized laser fields, which is interpreted as a result of strong birefringence of the gain medium near the wavelengths of the laser.

  18. On-Line/At-Line Technetium Monitor Using Scintillating Ion Exchange Resins for the Savannah River Site

    SciTech Connect

    Wach, S.T.

    2000-08-30

    The results of this study indicate that the combination of extraction chromatography and on-line flow-cell scintillation counting can exceed a 99Tc detection limit of 0.005 Ci/mL in the presence of 90Sr, 137Cs, and 239Pu in less than an 18 minute analysis time.

  19. Laser ion source activities at Brookhaven National Laboratory

    DOE PAGES

    Kanesue, Takeshi; Okamura, Masahiro

    2015-07-31

    In Brookhaven National Laboratory (BNL), we have been developing laser ion sources for diverse accelerators. Tabletop Nd:YAG lasers with up to several Joules of energy are mainly used to create ablation plasmas for stable operations. The obtained charge states depend on laser power density and target species. Two types of ion extraction schemes, Direct Plasma Injection Scheme (DPIS) and conventional static extraction, are used depending on application. We optimized and select a suitable laser irradiation condition and a beam extraction scheme to meet the requirement of the following accelerator system. We have demonstrated to accelerate more than 5 x 1010more » of C6+ ions using the DPIS. We successfully commissioned low charge ion beam provider to the user facilities in BNL. As a result, to achieve higher current, higher charge state and lower emittance, further studies will continue.« less

  20. Laser ion source activities at Brookhaven National Laboratory

    SciTech Connect

    Kanesue, Takeshi; Okamura, Masahiro

    2015-07-31

    In Brookhaven National Laboratory (BNL), we have been developing laser ion sources for diverse accelerators. Tabletop Nd:YAG lasers with up to several Joules of energy are mainly used to create ablation plasmas for stable operations. The obtained charge states depend on laser power density and target species. Two types of ion extraction schemes, Direct Plasma Injection Scheme (DPIS) and conventional static extraction, are used depending on application. We optimized and select a suitable laser irradiation condition and a beam extraction scheme to meet the requirement of the following accelerator system. We have demonstrated to accelerate more than 5 x 1010 of C6+ ions using the DPIS. We successfully commissioned low charge ion beam provider to the user facilities in BNL. As a result, to achieve higher current, higher charge state and lower emittance, further studies will continue.

  1. Early Clinical Experience With Argon Ion Laser Endarterectomy

    NASA Astrophysics Data System (ADS)

    Eugene, John; Baribeau, Yvon; Ott, Richard A.; McColgan, Stephen J.; Berns, Michael W.

    1989-09-01

    This report describes our progress in the development of argon ion laser endarterectomy for arteriosclerotic cardiovascular disease. Nine patients underwent 10 vascular reconstructions for claudication (6), rest pain (1), and gangrene (2). There was 1 aortoiliac endarterectomy, 6 superficial femoral artery endarterectomies, 1 profunda femoris endarterectomy and 2 popliteal endarterectomies. The reconstructions were 6 cm to 60 cm in length. The operations were performed using low power argon ion laser radiation, 1.0 W. All patients experienced symptomatic relief and had palpable pulses postoperatively. There were no perforations and there were no injuries to surrounding tissues from laser radiation. Surgical complications occurred and these were technical problems that should be eliminated from the operation with further developments. The early clinical results show that laser endarterectomy can be performed for peripheral vascular reconstruction using low power argon ion laser radiation.

  2. Low-Energy Ions from Laser-Cooled Atoms

    NASA Astrophysics Data System (ADS)

    Shayeganrad, G.; Fioretti, A.; Guerri, I.; Tantussi, F.; Ciampini, D.; Allegrini, M.; Viteau, M.; Fuso, F.

    2016-05-01

    We report the features of an ion source based on two-color photoionization of a laser-cooled cesium beam outsourced from a pyramidal magneto-optical trap. The ion source operates in continuous or pulsed mode. At acceleration voltages below 300 V, it delivers some ten ions per bunch with a relative energy spread Δ Urms/U ≃0.032 , as measured through the retarding field-energy-analyzer approach. Space-charge effects are negligible thanks to the low ion density attained in the interaction volume. The performances of the ion beam in a configuration using focused laser beams are extrapolated on the basis of the experimental results. Calculations demonstrate that our low-energy and low-current ion beam can be attractive for the development of emerging technologies requiring the delivery of a small amount of charge, down to the single-ion level and its eventual focusing in the 10-nm range.

  3. Emission Characteristics and Stability of Laser Ion Sources

    SciTech Connect

    Krasa, J.; Velyhan, A.; Krousky, E.; Laska, L.; Rohlena, K.; Jungwirth, K.; Ullschmied, J.; Lorusso, A.; Velardi, L.; Nassisi, V.; Czarnecka, A.; Ryc, L.; Parys, P.; Wolowksi, J.

    2010-10-13

    A new classification of laser ion sources concerning their pulse-to-pulse reproducibility in the ion emission is proposed. In particular, we distinguish between plasmas according to the electron distribution changing its characteristics at a laser intensity threshold of 10{sup 14} W/cm{sup 2}. Well reproducible continuous pulsed ion currents are typical for the intensity below the threshold. In contrast to this plasma the 'two-temperature' plasma arising for the intensity above this threshold shows not only a separation of charges in space and time but it also shows irregular and intense outbursts of ions similar to a self pulsing instability leading to a chaos. The sequence of fast ion outbursts visible on time-of-flight spectra is sensitive to details of non-linear interaction of the sub-nanosecond laser beam with the generated plasma.

  4. Laser desorption in an ion trap mass spectrometer

    SciTech Connect

    Eiden, G.C.; Cisper, M.E.; Alexander, M.L.; Hemberger, P.H.; Nogar, N.S.

    1993-02-01

    Laser desorption in a ion-trap mass spectrometer shows significant promise for both qualitative and trace analysis. Several aspects of this methodology are discussed in this work. We previously demonstrated the generation of both negative and positive ions by laser desorption directly within a quadrupole ion trap. In the present work, we explore various combinations of d.c., r.f., and time-varying fields in order to optimize laser generated signals. In addition, we report on the application of this method to analyze samples containing compounds such as amines, metal complexes, carbon clusters, and polynuclear aromatic hydrocarbons. In some cases the ability to rapidly switch between positive and negative ion modes provides sufficient specificity to distinguish different compounds of a mixture with a single stage of mass spectrometry. In other experiments, we combined intensity variation studies with tandem mass spectrometry experiments and positive and negative ion detection to further enhance specificity.

  5. Review of laser-driven ion sources and their applications.

    PubMed

    Daido, Hiroyuki; Nishiuchi, Mamiko; Pirozhkov, Alexander S

    2012-05-01

    For many years, laser-driven ion acceleration, mainly proton acceleration, has been proposed and a number of proof-of-principle experiments have been carried out with lasers whose pulse duration was in the nanosecond range. In the 1990s, ion acceleration in a relativistic plasma was demonstrated with ultra-short pulse lasers based on the chirped pulse amplification technique which can provide not only picosecond or femtosecond laser pulse duration, but simultaneously ultra-high peak power of terawatt to petawatt levels. Starting from the year 2000, several groups demonstrated low transverse emittance, tens of MeV proton beams with a conversion efficiency of up to several percent. The laser-accelerated particle beams have a duration of the order of a few picoseconds at the source, an ultra-high peak current and a broad energy spectrum, which make them suitable for many, including several unique, applications. This paper reviews, firstly, the historical background including the early laser-matter interaction studies on energetic ion acceleration relevant to inertial confinement fusion. Secondly, we describe several implemented and proposed mechanisms of proton and/or ion acceleration driven by ultra-short high-intensity lasers. We pay special attention to relatively simple models of several acceleration regimes. The models connect the laser, plasma and proton/ion beam parameters, predicting important features, such as energy spectral shape, optimum conditions and scalings under these conditions for maximum ion energy, conversion efficiency, etc. The models also suggest possible ways to manipulate the proton/ion beams by tailoring the target and irradiation conditions. Thirdly, we review experimental results on proton/ion acceleration, starting with the description of driving lasers. We list experimental results and show general trends of parameter dependences and compare them with the theoretical predictions and simulations. The fourth topic includes a review of

  6. Implementation of a neural network for digital pulse shape analysis on a FPGA for on-line identification of heavy ions

    NASA Astrophysics Data System (ADS)

    Jiménez, R.; Sánchez-Raya, M.; Gómez-Galán, J. A.; Flores, J. L.; Dueñas, J. A.; Martel, I.

    2012-05-01

    Pulse shape analysis techniques for the identification of heavy ions produced in nuclear reactions have been recently proposed as an alternative to energy loss and time of flight methods. However this technique requires a large amount of memory for storing the shapes of charge and current signals. We have implemented a hardware solution for fast on-line processing of the signals producing the relevant information needed for particle identification. Since the pulse shape analysis can be formulated in terms of a pattern recognition problem, a neural network has been implemented in a FPGA device. The design concept has been tested using 12,13C ions produced in heavy ion reactions. The actual latency of the system is about 20 μs when using a clock frequency of 50 MHz.

  7. Laser Driven Ion accelerators - current status and perspective

    SciTech Connect

    Zepf, M.; Robinson, A. P. L.

    2009-01-22

    The interaction of ultra-intense lasers with thin foil targets has recently emerged as a route to achieving extreme acceleration gradients and hence ultra-compact proton and ion accelerators. There are a number of distinct physical processes by which the protons/ions can be accelerated to energies in excess of 10 MeV. The recent development is discussed and a new mechanism--Radiation Pressure Acceleration is highlighted as a route to achieving efficient production of relativistic ions beams.

  8. Laser-generated waves and wakes in rotating ion crystals.

    PubMed

    Kriesel, J M; Bollinger, J J; Mitchell, T B; King, L B; Dubin, D H E

    2002-03-25

    Locally excited plasma waves are generated in a Coulomb crystal by "pushing" with radiation pressure on a rotating cloud of laser-cooled 9Be+ ions. The waves form a stationary wake that is directly imaged through the dependence of the ion fluorescence on Doppler shifts, and theoretical calculations in a slab geometry are shown to accurately reproduce these images. The technique demonstrates a new method of exciting and studying waves in cold ion clouds.

  9. Laser-driven ion acceleration from relativistically transparent nanotargets

    NASA Astrophysics Data System (ADS)

    Hegelich, B. M.; Pomerantz, I.; Yin, L.; Wu, H. C.; Jung, D.; Albright, B. J.; Gautier, D. C.; Letzring, S.; Palaniyappan, S.; Shah, R.; Allinger, K.; Hörlein, R.; Schreiber, J.; Habs, D.; Blakeney, J.; Dyer, G.; Fuller, L.; Gaul, E.; Mccary, E.; Meadows, A. R.; Wang, C.; Ditmire, T.; Fernandez, J. C.

    2013-08-01

    Here we present experimental results on laser-driven ion acceleration from relativistically transparent, overdense plasmas in the break-out afterburner (BOA) regime. Experiments were preformed at the Trident ultra-high contrast laser facility at Los Alamos National Laboratory, and at the Texas Petawatt laser facility, located in the University of Texas at Austin. It is shown that when the target becomes relativistically transparent to the laser, an epoch of dramatic acceleration of ions occurs that lasts until the electron density in the expanding target reduces to the critical density in the non-relativistic limit. For given laser parameters, the optimal target thickness yielding the highest maximum ion energy is one in which this time window for ion acceleration overlaps with the intensity peak of the laser pulse. A simple analytic model of relativistically induced transparency is presented for plasma expansion at the time-evolving sound speed, from which these times may be estimated. The maximum ion energy attainable is controlled by the finite acceleration volume and time over which the BOA acts.

  10. Ion-implanted planar-buried-heterostructure diode laser

    DOEpatents

    Brennan, Thomas M.; Hammons, Burrell E.; Myers, David R.; Vawter, Gregory A.

    1991-01-01

    A Planar-Buried-Heterostructure, Graded-Index, Separate-Confinement-Heterostructure semiconductor diode laser 10 includes a single quantum well or multi-quantum well active stripe 12 disposed between a p-type compositionally graded Group III-V cladding layer 14 and an n-type compositionally graded Group III-V cladding layer 16. The laser 10 includes an ion implanted n-type region 28 within the p-type cladding layer 14 and further includes an ion implanted p-type region 26 within the n-type cladding layer 16. The ion implanted regions are disposed for defining a lateral extent of the active stripe.

  11. Low charge state heavy ion production with sub-nanosecond laser.

    PubMed

    Kanesue, T; Kumaki, M; Ikeda, S; Okamura, M

    2016-02-01

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target.

  12. Low charge state heavy ion production with sub-nanosecond laser

    NASA Astrophysics Data System (ADS)

    Kanesue, T.; Kumaki, M.; Ikeda, S.; Okamura, M.

    2016-02-01

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target.

  13. On-line and post irradiation analysis of swift heavy ion induced modification of PMMA (polymethyl-methacrylate)

    NASA Astrophysics Data System (ADS)

    Hossain, U. H.; Lima, V.; Baake, O.; Severin, D.; Bender, M.; Ensinger, W.

    2014-05-01

    The present work is part of a research program studying the swift heavy ion induced modification of aliphatic polymers with some comparable side groups, here polymethyl-methacrylate (PMMA). This paper presents a study on Fourier-transform-infrared spectroscopy (FTIR), residual gas analysis (RGA), and Ultraviolet-Visible (UV-Vis) spectroscopy of the transformations of a PMMA film under gold (Au) and uranium (U) ion irradiation in the MeV/u range in vacuum to fluences up to 3 × 1011 ions per cm2. The results show a general ion induced degradation of the polymer, with release of volatile fragments, scission of side chains and polymeric backbone, formation of conjugated double bonds, and the resulting increased absorption of the UV part in the UV-Vis spectral region. A molecular scission mechanism which explains the main degradation products is proposed.

  14. Tandem ion mobility spectrometry coupled to laser excitation

    SciTech Connect

    Simon, Anne-Laure; Choi, Chang Min; Clavier, Christian; Barbaire, Marc; Maurelli, Jacques; Dagany, Xavier; MacAleese, Luke; Dugourd, Philippe; Chirot, Fabien

    2015-09-15

    This manuscript describes a new experimental setup that allows to perform tandem ion mobility spectrometry (IMS) measurements and which is coupled to a high resolution time-of-flight mass spectrometer. It consists of two 79 cm long drift tubes connected by a dual ion funnel assembly. The setup was built to permit laser irradiation of the ions in the transfer region between the two drift tubes. This geometry allows selecting ions according to their ion mobility in the first drift tube, to irradiate selected ions, and examine the ion mobility of the product ions in the second drift tube. Activation by collision is possible in the same region (between the two tubes) and between the second tube and the time-of-flight. IMS-IMS experiments on Ubiquitin are reported. We selected a given isomer of charge state +7 and explored its structural rearrangement following collisional activation between the two drift tubes. An example of IMS-laser-IMS experiment is reported on eosin Y, where laser irradiation was used to produce radical ions by electron photodetachment starting from doubly deprotonated species. This allowed measuring the collision cross section of the radical photo-product, which cannot be directly produced with an electrospray source.

  15. Tandem ion mobility spectrometry coupled to laser excitation.

    PubMed

    Simon, Anne-Laure; Chirot, Fabien; Choi, Chang Min; Clavier, Christian; Barbaire, Marc; Maurelli, Jacques; Dagany, Xavier; MacAleese, Luke; Dugourd, Philippe

    2015-09-01

    This manuscript describes a new experimental setup that allows to perform tandem ion mobility spectrometry (IMS) measurements and which is coupled to a high resolution time-of-flight mass spectrometer. It consists of two 79 cm long drift tubes connected by a dual ion funnel assembly. The setup was built to permit laser irradiation of the ions in the transfer region between the two drift tubes. This geometry allows selecting ions according to their ion mobility in the first drift tube, to irradiate selected ions, and examine the ion mobility of the product ions in the second drift tube. Activation by collision is possible in the same region (between the two tubes) and between the second tube and the time-of-flight. IMS-IMS experiments on Ubiquitin are reported. We selected a given isomer of charge state +7 and explored its structural rearrangement following collisional activation between the two drift tubes. An example of IMS-laser-IMS experiment is reported on eosin Y, where laser irradiation was used to produce radical ions by electron photodetachment starting from doubly deprotonated species. This allowed measuring the collision cross section of the radical photo-product, which cannot be directly produced with an electrospray source.

  16. Note: A pulsed laser ion source for linear induction accelerators

    NASA Astrophysics Data System (ADS)

    Zhang, H.; Zhang, K.; Shen, Y.; Jiang, X.; Dong, P.; Liu, Y.; Wang, Y.; Chen, D.; Pan, H.; Wang, W.; Jiang, W.; Long, J.; Xia, L.; Shi, J.; Zhang, L.; Deng, J.

    2015-01-01

    We have developed a high-current laser ion source for induction accelerators. A copper target was irradiated by a frequency-quadrupled Nd:YAG laser (266 nm) with relatively low intensities of 108 W/cm2. The laser-produced plasma supplied a large number of Cu+ ions (˜1012 ions/pulse) during several microseconds. Emission spectra of the plasma were observed and the calculated electron temperature was about 1 eV. An induction voltage adder extracted high-current ion beams over 0.5 A/cm2 from a plasma-prefilled gap. The normalized beam emittance measured by a pepper-pot method was smaller than 1 π mm mrad.

  17. Note: A pulsed laser ion source for linear induction accelerators

    SciTech Connect

    Zhang, H.; Zhang, K.; Shen, Y.; Jiang, X.; Dong, P.; Liu, Y.; Wang, Y.; Chen, D.; Pan, H.; Wang, W.; Jiang, W.; Long, J.; Xia, L.; Shi, J.; Zhang, L.; Deng, J.

    2015-01-15

    We have developed a high-current laser ion source for induction accelerators. A copper target was irradiated by a frequency-quadrupled Nd:YAG laser (266 nm) with relatively low intensities of 10{sup 8} W/cm{sup 2}. The laser-produced plasma supplied a large number of Cu{sup +} ions (∼10{sup 12} ions/pulse) during several microseconds. Emission spectra of the plasma were observed and the calculated electron temperature was about 1 eV. An induction voltage adder extracted high-current ion beams over 0.5 A/cm{sup 2} from a plasma-prefilled gap. The normalized beam emittance measured by a pepper-pot method was smaller than 1 π mm mrad.

  18. Multiple Ionization Bursts in Laser-Driven Hydrogen Molecular Ion

    SciTech Connect

    Takemoto, Norio; Becker, Andreas

    2010-11-12

    Theoretical study on H{sub 2}{sup +} in an intense infrared laser field on the attosecond time scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely accepted tunnel ionization picture for an atom. These bursts are found to be induced by transient localization of the electron at one of the nuclei, and a relation between the time instants of the localization and the vector potential of the laser light is derived. A scheme is proposed to probe the localization dynamics by an extreme ultraviolet laser pulse.

  19. Tunable diode laser absorption spectroscopy-based tomography system for on-line monitoring of two-dimensional distributions of temperature and H2O mole fraction

    NASA Astrophysics Data System (ADS)

    Xu, Lijun; Liu, Chang; Jing, Wenyang; Cao, Zhang; Xue, Xin; Lin, Yuzhen

    2016-01-01

    To monitor two-dimensional (2D) distributions of temperature and H2O mole fraction, an on-line tomography system based on tunable diode laser absorption spectroscopy (TDLAS) was developed. To the best of the authors' knowledge, this is the first report on a multi-view TDLAS-based system for simultaneous tomographic visualization of temperature and H2O mole fraction in real time. The system consists of two distributed feedback (DFB) laser diodes, a tomographic sensor, electronic circuits, and a computer. The central frequencies of the two DFB laser diodes are at 7444.36 cm-1 (1343.3 nm) and 7185.6 cm-1 (1391.67 nm), respectively. The tomographic sensor is used to generate fan-beam illumination from five views and to produce 60 ray measurements. The electronic circuits not only provide stable temperature and precise current controlling signals for the laser diodes but also can accurately sample the transmitted laser intensities and extract integrated absorbances in real time. Finally, the integrated absorbances are transferred to the computer, in which the 2D distributions of temperature and H2O mole fraction are reconstructed by using a modified Landweber algorithm. In the experiments, the TDLAS-based tomography system was validated by using asymmetric premixed flames with fixed and time-varying equivalent ratios, respectively. The results demonstrate that the system is able to reconstruct the profiles of the 2D distributions of temperature and H2O mole fraction of the flame and effectively capture the dynamics of the combustion process, which exhibits good potential for flame monitoring and on-line combustion diagnosis.

  20. Numerical analysis of 50 Gbaud homodyne coherent receivers relying on line-coding and injection locking in lasers

    NASA Astrophysics Data System (ADS)

    Xydas, Yannis; Ressopoulos, Constantinos; Bogris, Adonis

    2015-12-01

    We present a numerical analysis of 50 Gbaud coherent detection enabled by injection locked lasers and line coding. The coherent receiver was tested with respect to an ideal receiver for two higher order modulation formats (16-QAM, QPSK) and under diverse operating regimes relating to the slave laser linewidth properties, the injection level and the frequency detuning between the incoming signal and the slave laser. The impact of the slave laser properties and line coding techniques on the receiver performance is highlighted showing that the technique could be used as a practical solution in order to enable low-cost and short reach n × 100 Gb/s Ethernet communication systems with the potential of flexibility in terms of the data rate.

  1. Storage of ions from laser-produced plasmas

    NASA Technical Reports Server (NTRS)

    Knight, R. D.

    1981-01-01

    A method of storing large numbers of metal ions created in laser-produced plasmas is presented. The outer electrode of the electrostatic ion trap is designed to give a harmonic axial potential. The ions trapped by the technique included Be(+), C(+), Al(+), Fe(+), and Pb(+). The initial number of ions stored (2 x 10 to the 8th) appeared to be the trap maximum since increasing the laser power beyond 2-3 MW did not change the ion number. An initial rapid decay in the 30-50 msec range was generally followed by a long tail at the 10% level with times greater than 100 msec. The technique should be valuable for refractory elements which cannot be easily vaporized for electron impact ionization.

  2. Ion acceleration from laser-driven electrostatic shocks

    SciTech Connect

    Fiuza, F.; Stockem, A.; Boella, E.; Fonseca, R. A.; Silva, L. O.; Haberberger, D.; Tochitsky, S.; Mori, W. B.; Joshi, C.

    2013-05-15

    Multi-dimensional particle-in-cell simulations are used to study the generation of electrostatic shocks in plasma and the reflection of background ions to produce high-quality and high-energy ion beams. Electrostatic shocks are driven by the interaction of two plasmas with different density and/or relative drift velocity. The energy and number of ions reflected by the shock increase with increasing density ratio and relative drift velocity between the two interacting plasmas. It is shown that the interaction of intense lasers with tailored near-critical density plasmas allows for the efficient heating of the plasma electrons and steepening of the plasma profile at the critical density interface, leading to the generation of high-velocity shock structures and high-energy ion beams. Our results indicate that high-quality 200 MeV shock-accelerated ion beams required for medical applications may be obtained with current laser systems.

  3. Development of C⁶⁺ laser ion source and RFQ linac for carbon ion radiotherapy.

    PubMed

    Sako, T; Yamaguchi, A; Sato, K; Goto, A; Iwai, T; Nayuki, T; Nemoto, K; Kayama, T; Takeuchi, T

    2016-02-01

    A prototype C(6+) injector using a laser ion source has been developed for a compact synchrotron dedicated to carbon ion radiotherapy. The injector consists of a laser ion source and a 4-vane radio-frequency quadrupole (RFQ) linac. Ion beams are extracted from plasma and directly injected into the RFQ. A solenoid guides the low-energy beams into the RFQ. The RFQ is designed to accelerate high-intensity pulsed beams. A structure of monolithic vanes and cavities is adopted to reduce its power consumption. In beam acceleration tests, a solenoidal magnetic field set between the laser ion source and the RFQ helped increase both the peak currents before and after the RFQ by a factor of 4. PMID:26932119

  4. Development of C⁶⁺ laser ion source and RFQ linac for carbon ion radiotherapy.

    PubMed

    Sako, T; Yamaguchi, A; Sato, K; Goto, A; Iwai, T; Nayuki, T; Nemoto, K; Kayama, T; Takeuchi, T

    2016-02-01

    A prototype C(6+) injector using a laser ion source has been developed for a compact synchrotron dedicated to carbon ion radiotherapy. The injector consists of a laser ion source and a 4-vane radio-frequency quadrupole (RFQ) linac. Ion beams are extracted from plasma and directly injected into the RFQ. A solenoid guides the low-energy beams into the RFQ. The RFQ is designed to accelerate high-intensity pulsed beams. A structure of monolithic vanes and cavities is adopted to reduce its power consumption. In beam acceleration tests, a solenoidal magnetic field set between the laser ion source and the RFQ helped increase both the peak currents before and after the RFQ by a factor of 4.

  5. Laser desorption lamp ionization source for ion trap mass spectrometry.

    PubMed

    Wu, Qinghao; Zare, Richard N

    2015-01-01

    A two-step laser desorption lamp ionization source coupled to an ion trap mass spectrometer (LDLI-ITMS) has been constructed and characterized. The pulsed infrared (IR) output of an Nd:YAG laser (1064 nm) is directed to a target inside a chamber evacuated to ~15 Pa causing desorption of molecules from the target's surface. The desorbed molecules are ionized by a vacuum ultraviolet (VUV) lamp (filled with xenon, major wavelength at 148 nm). The resulting ions are stored and detected in a three-dimensional quadrupole ion trap modified from a Finnigan Mat LCQ mass spectrometer operated at a pressure of ≥ 0.004 Pa. The limit of detection for desorbed coronene molecules is 1.5 pmol, which is about two orders of magnitude more sensitive than laser desorption laser ionization mass spectrometry using a fluorine excimer laser (157 nm) as the ionization source. The mass spectrum of four standard aromatic compounds (pyrene, coronene, rubrene and 1,4,8,11,15,18,22,25-octabutoxy-29H,31H-phthalocyanine (OPC)) shows that parent ions dominate. By increasing the infrared laser power, this instrument is capable of detecting inorganic compounds. PMID:25601688

  6. Ion Beam Analysis applied to laser-generated plasmas

    NASA Astrophysics Data System (ADS)

    Cutroneo, M.; Macková, A.; Havranek, V.; Malinsky, P.; Torrisi, L.; Kormunda, M.; Barchuk, M.; Ullschmied, J.; Dudzak, R.

    2016-04-01

    This paper presents the research activity on Ion Beam Analysis methods performed at Tandetron Laboratory (LT) of the Institute of Nuclear Physics AS CR, Rez, Czech Republic. Recently, many groups are paying attention to implantation by laser generated plasma. This process allows to insert a controllable amount of energetic ions into the surface layers of different materials modifying the physical and chemical properties of the surface material. Different substrates are implanted by accelerated ions from plasma through terawatt iodine laser, at nominal intensity of 1015 W/cm2, at the PALS Research Infrastructure AS CR, in the Czech Republic. This regime of the laser matter interaction generates, multi-MeV proton beams, and multi-charged ions that are tightly confined in time (hundreds ps) and space (source radius of a few microns). These ion beams have a much lower transverse temperature, a much shorter duration and a much higher current than those obtainable from conventional accelerators. The implementation of protons and ions acceleration driven by ultra-short high intensity lasers is exhibited by adopting suitable irradiation conditions as well as tailored targets. An overview of implanted targets and their morphological and structural characterizations is presented and discussed.

  7. [Determination of trace and ultra-trace level bromate in water by large volume sample injection with enrichment column for on-line preconcentration coupled with ion chromatography].

    PubMed

    Liu, Jing; He, Qingqing; Yang, Lili; Hu, Enyu; Wang, Meifei

    2015-10-01

    A method for the determination of trace and ultra-trace level bromate in water by ion chromatography with large volume sample injection for on-line preconcentration was established. A high capacity Dionex IonPac AG23 guard column was simply used as the enrichment column instead of the loop for the preconcentration of bromate. High purity KOH solution used as eluent for gradient elution was on-line produced by an eluent generator automatically. The results showed that a good linear relationship of bromate was exhibited in the range of 0.05-51.2 μg/L (r ≥ 0.999 5), and the method detection limit was 0.01 μg/L. Compared with conventional sample injection, the injection volume was up to 5 mL, and the enrichment factor of this method was about 240 times. This method was successfully applied for several real samples of pure water which were purchased in the supermarket, and the recoveries of bromate were between 90%-100% with the RSDs (n = 6) of 2.1%-6.4% at two spiked levels. This method without pretreatment is simple, and of high accuracy and precision. The preconcentration can be achieved by large volume sample injection. It is suitable for the analysis of trace and ultra-trace level bromate.

  8. Development of a large depth of field collection optics for on-line Laser-Induced Breakdown Spectroscopy applications

    NASA Astrophysics Data System (ADS)

    Redoglio, Daniele A.; Golinelli, Elena; Musazzi, Sergio; Perini, Umberto; Barberis, Franco

    2016-09-01

    This paper deals with the study of the collection optics required by a LIBS system that has to perform on-line analysis of moving samples whose distance may vary during measurements. Main requirement of this system is to maintain good collection efficiency over a wide range of sample distances by using a fixed focus optical arrangement. The selected configuration is based on the use of two spherical mirrors with the same curvature radius. Tests carried out on an experimental prototype are in good agreement with the previously performed simulations.

  9. Design of a laser-induced breakdown spectroscopy system for on-line quality analysis of pulverized coal in power plants

    SciTech Connect

    Yin, W.B.; Zhang, L.; Dong, L.; Ma, W.G.; Jia, S.T.

    2009-08-15

    It is vitally important for a power plant to determine the chemical composition of coal prior to combustion in order to obtain optimal boiler control. In this work, a fully software-controlled laser-induced breakdown spectroscopy (LIBS) system comprising a LIBS apparatus and sampling equipment has been designed for possible application to power plants for on-line quality analysis of pulverized coal. Special attention was given to the LIBS system, the data processing methods (especially the normalization with Bode Rule/DC Level) and the specific settings (the software-controlled triggering source, high-pressure gas cleaning device, sample preparation module, sampling module, etc.), which gave the best direct measurement for C, H, Si, Na, Mg, Fe, Al, and Ti with measurement errors less than 10% for pulverized coal. Therefore, the apparatus is accurate enough to be applied to industries for on-line monitoring of pulverized coal. The method of proximate analysis was also introduced and the experimental error of A(ad) (Ash, 'ad' is an abbreviation for 'air dried') was shown in the range of 2.29 to 13.47%. The programmable logic controller (PLC) controlled on-line coal sampling equipment, which is designed based upon aerodynamics, and is capable of performing multipoint sampling and sample-preparation operation.

  10. Design of a laser-induced breakdown spectroscopy system for on-line quality analysis of pulverized coal in power plants.

    PubMed

    Yin, Wangbao; Zhang, Lei; Dong, Lei; Ma, Weiguang; Jia, Suotang

    2009-08-01

    It is vitally important for a power plant to determine the chemical composition of coal prior to combustion in order to obtain optimal boiler control. In this work, a fully software-controlled laser-induced breakdown spectroscopy (LIBS) system comprising a LIBS apparatus and sampling equipment has been designed for possible application to power plants for on-line quality analysis of pulverized coal. Special attention was given to the LIBS system, the data processing methods (especially the normalization with Bode Rule/DC Level) and the specific settings (the software-controlled triggering source, high-pressure gas cleaning device, sample-preparation module, sampling module, etc.), which gave the best direct measurement for C, H, Si, Na, Mg, Fe, Al, and Ti with measurement errors less than 10% for pulverized coal. Therefore, the apparatus is accurate enough to be applied to industries for on-line monitoring of pulverized coal. The method of proximate analysis was also introduced and the experimental error of A(ad) (Ash, 'ad' is an abbreviation for 'air dried') was shown in the range of 2.29 to 13.47%. The programmable logic controller (PLC) controlled on-line coal sampling equipment, which is designed based upon aerodynamics, and is capable of performing multipoint sampling and sample-preparation operation.

  11. Chirped-Standing-Wave Acceleration of Ions with Intense Lasers.

    PubMed

    Mackenroth, F; Gonoskov, A; Marklund, M

    2016-09-01

    We propose a novel mechanism for ion acceleration based on the guided motion of electrons from a thin layer. The electron motion is locked to the moving nodes of a standing wave formed by a chirped laser pulse reflected from a mirror behind the layer. This provides a stable longitudinal field of charge separation, thus giving rise to chirped-standing-wave acceleration of the residual ions of the layer. We demonstrate, both analytically and numerically, that stable proton beams, with energy spectra peaked around 100 MeV, are feasible for pulse energies at the level of 10 J. Moreover, a scaling law for higher laser intensities and layer densities is presented, indicating stable GeV-level energy gains of dense ion bunches, for soon-to-be-available laser intensities. PMID:27636480

  12. Plasma shape control by pulsed solenoid on laser ion source

    DOE PAGES

    Sekine, M.; Ikeda, S.; Romanelli, M.; Kumaki, M.; Fuwa, Y.; Kanesue, T.; Hayashizaki, N.; Lambiase, R.; Okamura, M.

    2015-05-28

    A Laser ion source (LIS) provides high current heavy ion beams with a very simple mechanical structure. Plasma is produced by a pulsed laser ablation of a solid state target and ions are extracted by an electric field. It was difficult to manipulate the beam parameters of a LIS, since the plasma condition could only be adjusted by the laser irradiation condition. To enhance flexibility of LIS operation, we employed a pulsed solenoid in the plasma drift section and investigated the effect of the solenoid field on singly charged iron beams. The experimentally obtained current profile was satisfactorily controlled bymore » the pulsed magnetic field. Thus, this approach may also be useful to reduce beam emittance of a LIS.« less

  13. Plasma shape control by pulsed solenoid on laser ion source

    SciTech Connect

    Sekine, M.; Ikeda, S.; Romanelli, M.; Kumaki, M.; Fuwa, Y.; Kanesue, T.; Hayashizaki, N.; Lambiase, R.; Okamura, M.

    2015-05-28

    A Laser ion source (LIS) provides high current heavy ion beams with a very simple mechanical structure. Plasma is produced by a pulsed laser ablation of a solid state target and ions are extracted by an electric field. It was difficult to manipulate the beam parameters of a LIS, since the plasma condition could only be adjusted by the laser irradiation condition. To enhance flexibility of LIS operation, we employed a pulsed solenoid in the plasma drift section and investigated the effect of the solenoid field on singly charged iron beams. The experimentally obtained current profile was satisfactorily controlled by the pulsed magnetic field. Thus, this approach may also be useful to reduce beam emittance of a LIS.

  14. Chirped-Standing-Wave Acceleration of Ions with Intense Lasers.

    PubMed

    Mackenroth, F; Gonoskov, A; Marklund, M

    2016-09-01

    We propose a novel mechanism for ion acceleration based on the guided motion of electrons from a thin layer. The electron motion is locked to the moving nodes of a standing wave formed by a chirped laser pulse reflected from a mirror behind the layer. This provides a stable longitudinal field of charge separation, thus giving rise to chirped-standing-wave acceleration of the residual ions of the layer. We demonstrate, both analytically and numerically, that stable proton beams, with energy spectra peaked around 100 MeV, are feasible for pulse energies at the level of 10 J. Moreover, a scaling law for higher laser intensities and layer densities is presented, indicating stable GeV-level energy gains of dense ion bunches, for soon-to-be-available laser intensities.

  15. Chirped-Standing-Wave Acceleration of Ions with Intense Lasers

    NASA Astrophysics Data System (ADS)

    Mackenroth, F.; Gonoskov, A.; Marklund, M.

    2016-09-01

    We propose a novel mechanism for ion acceleration based on the guided motion of electrons from a thin layer. The electron motion is locked to the moving nodes of a standing wave formed by a chirped laser pulse reflected from a mirror behind the layer. This provides a stable longitudinal field of charge separation, thus giving rise to chirped-standing-wave acceleration of the residual ions of the layer. We demonstrate, both analytically and numerically, that stable proton beams, with energy spectra peaked around 100 MeV, are feasible for pulse energies at the level of 10 J. Moreover, a scaling law for higher laser intensities and layer densities is presented, indicating stable GeV-level energy gains of dense ion bunches, for soon-to-be-available laser intensities.

  16. Towards Laser Cooling Trapped Ions with Telecom Light

    NASA Astrophysics Data System (ADS)

    Dungan, Kristina; Becker, Patrick; Donoghue, Liz; Liu, Jackie; Olmschenk, Steven

    2015-05-01

    Quantum information has many potential applications in communication, atomic clocks, and the precision measurement of fundamental constants. Trapped ions are excellent candidates for applications in quantum information because of their isolation from external perturbations, and the precise control afforded by laser cooling and manipulation of the quantum state. For many applications in quantum communication, it would be advantageous to interface ions with telecom light. We present progress towards laser cooling and trapping of doubly-ionized lanthanum, which should require only infrared, telecom-compatible light. Additionally, we present progress on optimization of a second-harmonic generation cavity for laser cooling and trapping barium ions, for future sympathetic cooling experiments. This research is supported by the Army Research Office, Research Corporation for Science Advancement, and Denison University.

  17. Quantification Of Cesium In Negative Hydrogen Ion Sources By Laser Absorption Spectroscopy

    SciTech Connect

    Fantz, U.; Wimmer, Ch.

    2011-09-26

    The use of cesium in negative hydrogen ion sources and the resulting cesium dynamics caused by the evaporation and redistribution in the vacuum and plasma phase makes a reliable and on-line monitoring of the cesium amount in the source highly desirable. For that purpose, a robust and compact laser absorption setup suitable for the ion source environment has been developed utilizing the Cs D{sub 2} resonance line at 852.1 nm. First measurements are taken in a small laboratory plasma chamber with cesium evaporation. A detection limit of {approx_equal}5x10{sup 13} m{sup -3} at a typical path length of 15 cm has been obtained with a dynamic range of more than three orders of magnitude, limited by line saturation at high densities. For on-line monitoring an automatic data analysis is established achieving a temporal resolution of 100 ms. The setup has then been applied to the ITER prototype ion sources developed at IPP. It is been shown that the method is well suited for routine measurements revealing a new insight into the cesium dynamics during source operation and cesium conditioning.

  18. Bound state - excitation in ion-ion collisions related to X-ray lasers modelling

    SciTech Connect

    Stancalie, V.; Sureau, A.; Klisnick, A.

    1995-12-31

    As in the earlier work of Walling and Weisheit we used the Seaton`s semi-classical, impact parameter formulation of Coulomb excitation for a variety of inelastic ion-ion collisions, involved in laser-produced soft X-ray lasers with Li-like aluminum ions, 1s{sup 2} nl configuration. Energy levels has been calculated by direct SCF method including the spin-orbit interaction. Our definition of the electric 2{sup {lambda}} - pole line strength, S{sup {lambda}}, is consistent with that of Sobelman. The ion-ion collision processes have been considered for a wide range of temperature between 500 eV to 30 eV, with a particular interest in the last part of plasma evolution time, when complications such as non-Maxwellian particle distributions, radiation fields and transient plasma conditions can be neglected, and when the plasma electrons and ions have comparable temperatures.

  19. Laser ion source with solenoid for Brookhaven National Laboratory-electron beam ion source.

    PubMed

    Kondo, K; Yamamoto, T; Sekine, M; Okamura, M

    2012-02-01

    The electron beam ion source (EBIS) preinjector at Brookhaven National Laboratory (BNL) is a new heavy ion-preinjector for relativistic heavy ion collider (RHIC) and NASA Space Radiation Laboratory (NSRL). Laser ion source (LIS) is a primary ion source provider for the BNL-EBIS. LIS with solenoid at the plasma drift section can realize the low peak current (∼100 μA) with high charge (∼10 nC) which is the BNL-EBIS requirement. The gap between two solenoids does not cause serious plasma current decay, which helps us to make up the BNL-EBIS beamline.

  20. Laser Cooled Strontium Source for an Ion Interferometer

    NASA Astrophysics Data System (ADS)

    Lyon, Mary; Archibald, James; Erickson, Christopher; Durfee, Dallin

    2010-10-01

    We present a Strontium-87 magneto-optical trap (MOT) in a Low-Velocity-Intense-Source (LVIS) as the source of cooled, collimated atoms for an ion interferometer. Laser cooling and trapping is accomplished with a 461 nm frequency doubled laser and a pair of permanent magnets. A beam of cooled atoms is produced by passing the atoms through a hole drilled in one of the retroreflecting optics. The atoms are then photo-ionized in a two photon process.

  1. On-Line Derivatization Gas Chromatography Ion Trap Mass Spectrometry for Determination of Endocrine Disruptors in Surface Water

    SciTech Connect

    Tzing, Shin-Hwa; Chang, Jia-Yaw; Ling, Yong-Chien

    2004-03-31

    A method has been developed for the determination of endocrine disruptors (EDs) (containing hydroxyl groups) in surface water from different sources. The surface water samples from different sites including school and local dormitory sewage effluents, lake water and river water were collected and analyzed. In this method, the pretreated sample is directly analyzed by GC-MS using on-line derivatization, where tetramethylammonium hydroxide (TMA-OH) was used as the derivatizing agent. Use of large-volume direct sample introduction (DSI) and co-injection of the sample and TMAOH avoids external contaminations as observed in conventional derivatization protocols. Additionally, the use of chemical ionization (CI) and CI-MS/MS could enable detection of EDs at lower concentrations and reduce the matrices' interference thereby enhancing detection sensitivity of EDs for quantification. In this work, the use of dichloromethane as CI reagent for EDs is reported for the first time and could detect EDs to concentrations as low as 0.5 pg/mL. The recovery ranged from 74 to 112 % and the relative standard derivations for replicate analyses ranged from 5 to 17 %. We hope that this method will be applicable for routine analysis of EDs with hydroxyl functional groups.

  2. Is laser cooling for heavy-ion fusion feasible?

    NASA Astrophysics Data System (ADS)

    Ho, D. D.-M.; Brandon, S. T.

    2010-12-01

    Heavy-ion beams, each with current in the kiloampere range and particle energy in the giga-electronvolt range, must be focused onto a millimetre-size spot to provide the power required for ignition of high-gain targets for inertial confinement fusion. However, the focal spot size is always enlarged by chromatic aberration generated by the thermal spread of the beam ions in the direction of beam propagation. Enlarged focal spot degrades the target performance. For high-current beams, the conventional remedy for chromatic aberration using sextupole magnets has been shown to be ineffective. If novel correction schemes can be found, then the spot size can be reduced to below that previously believed possible. Smaller spots can mean lower energy targets so that the heavy-ion fusion (HIF) scenario can look more attractive. Success in laser cooling of ion beams in storage rings has inspired us to explore the feasibility of applying laser cooling for HIF, and the recirculator configuration proposed for HIF appears to be well suited for this purpose. However, using particle-in-cell simulations and theoretical arguments, we demonstrate in this paper that although laser cooling of heavy-ion beams is feasible in principle, the rapid velocity-space diffusion of ions in the bump-in-tail distribution, set up by the cooling lasers, limits the velocity-space compressibility of the thermal spread along the beam. Consequently, laser cooling is impractical for high-current, heavy-ion beams for the proposed recirculator configuration. Nevertheless, if the recirculator architecture or the target requirement can reduce the beam current, then the cooling scheme described here would be useful. This scheme may also be applicable to the RF linac and storage ring approach to HIF.

  3. Laser-ion acceleration through controlled surface contamination

    SciTech Connect

    Hou Bixue; Nees, John A.; He Zhaohan; Easter, James H.; Thomas, Alexander G. R.; Krushelnick, Karl M.; Petrov, George; Davis, Jack

    2011-04-15

    In laser-plasma ion accelerators, control of target contamination layers can lead to selection of accelerated ion species and enhancement of acceleration. To demonstrate this, deuterons up to 75 keV are accelerated from an intense laser interaction with a glass target simply by placing 1 ml of heavy water inside the experimental chamber prior to pumping to generate a deuterated contamination layer on the target. Using the same technique with a deuterated-polystyrene-coated target also enhances deuteron yield by a factor of 3 to 5, while increasing the maximum energy of the generated deuterons to 140 keV.

  4. Direct ion acceleration with variable-frequency lasers

    NASA Astrophysics Data System (ADS)

    Peano, Fabio; Vieira, Jorge; Fonseca, Ricardo; Silva, Luis; Coppa, Gianni; Mulas, Roberta

    2007-11-01

    Laser-based ion acceleration commonly relies on indirect schemes, in which the ions are accelerated by the space-charge field in laser-irradiated solid targets, either via plasma-expansion processes [1], or resorting to electrostatic shock structures [2]. Here, we propose the production of monoergetic ion beams via direct acceleration by the laser field (in vacuum or in tenuous plasmas) [3]. The method exploits two counterpropagating lasers with variable frequency to drive a beat-wave structure with variable phase velocity: the ions are trapped in the beat wave and accelerated to high energies. The physical mechanism is described with a 1D theory, providing the general conditions for trapping and scaling laws for the relevant ion-beam features. The validity and the robustness of the method are confirmed by 2D PIC simulations with OSIRIS [4]. [1] J. Fuchs et al., Nature Phys. 2, 48 (2006); L. Robson et al., Nature Phys. 3, 58 (2007); B.M. Hegelich et al., Nature 439, 441 (2006). [2] L.O. Silva et al., Phys. Rev. Lett. 92, 015002 (2004). [3] F. Peano et al., submitted for publication (2007). [4] R. A. Fonseca et al., Lect. Notes Comp. Sci. 2331, 342 (Springer-Verlag, Heidelberg, 2002).

  5. The beat in laser-accelerated ion beams

    SciTech Connect

    Schnürer, M.; Abicht, F.; Bränzel, J.; Koschitzki, Ch.; Andreev, A. A.; Platonov, K. Yu.; Priebe, G.; Sandner, W.

    2013-10-15

    Regular modulation in the ion velocity distribution becomes detectable if intense femtosecond laser pulses with very high temporal contrast are used for target normal sheath acceleration of ions. Analytical and numerical analysis of the experimental observation associates the modulation with the half-cycle of the driving laser field period. In processes like ion acceleration, the collective and laser-frequency determined electron dynamics creates strong fields in plasma to accelerate the ions. Even the oscillatory motion of electrons and its influence on the acceleration field can dominate over smoothing effects in plasma if a high temporal contrast of the driving laser pulse is given. Acceleration parameters can be directly concluded out of the experimentally observed modulation period in ion velocity spectra. The appearance of the phenomenon at a temporal contrast of ten orders between the intensity of the pulse peak and the spontaneous amplified emission background as well as remaining intensity wings at picosecond time-scale might trigger further parameter studies with even higher contrast.

  6. Production of He-like light and medium mass ions in laser ion source

    NASA Astrophysics Data System (ADS)

    Kondrashev, S.; Mescheryakov, N.; Sharkov, B.; Shumshurov, A.; Khomenko, S.; Makarov, K.; Satov, Yu.; Smakovskii, Yu.

    2000-03-01

    Operation of the laser ion source of He-like light ions designed for the first stage of the ITEP Terra Watt Accumulator (TWAC) project is discussed. A 5 J/0.5 Hz rep-rate CO2 laser was used for generation of highly charged light ions. The absolute number of ions with different charge states for carbon and aluminum ion beams has been measured. The obtained number of C+4 ions (˜1011ions/pulse) is sufficient to start the experimental proof of the accelerator scheme of the TWAC project. The investigation of shot to shot stability indicates significant increasing (˜2-3 times) of highly charged ion yield for the first shot onto the fresh target surface with respect to the next shots onto the same spot of aluminum target. This effect was not observed for the carbon target. Experimental results for highly charged light and medium mass (F, Mg, Al, Ca, Ti) ions produced by of 75 J single pulse CO2 laser consisting of a master oscillator and power amplifier are also presented.

  7. Laser generation of Au ions with charge states above 50+

    SciTech Connect

    Laska, L.; Jungwirth, K.; Krasa, J.; Krousky, E.; Rohlena, K.; Skala, J.; Velyhan, A.; Margarone, D.; Torrisi, L.; Ryc, L.; Ullschmied, J.

    2008-02-15

    Results of recent studies on highly charged Au ion generation, using the intense long pulses of the PALS high power iodine laser ({lambda}=1.315 {mu}m, E{sub L}=800 J/400 ps), operating under variable experimental conditions (1{omega}, 3{omega}, varying target thickness and changing focus positions), are presented. Both the ion collectors and the ion electrostatic analyzers were applied for the identification of ions in a large distance from the target. The time-of-flight collector signals were treated by a means of peak deconvolution assuming a shifted Maxwell-Boltzmann form of the constituent ion current peaks. Attention was paid to the influence of pulse precursor, which becomes evident, especially, if using thinner targets and 1{omega}. The results for 3{omega} point to the presence of several groups of ions with the highest recorded charge state Au{sup 53+}.

  8. Coulomb expansion of laser-excited ion plasmas.

    PubMed

    Feldbaum, D; Morrow, N V; Dutta, S K; Raithel, G

    2002-10-21

    We determine the electric field in mm-sized clouds of cold Rb+ ions, produced by photoionization of laser-cooled 87Rb atoms in a magneto-optical trap, using the Stark effect of embedded Rydberg atoms. The dependence of the electric field on the time delay between the ion plasma production and the probe of the electric field reflects the Coulomb expansion of the plasma. Our experiments and models show expansion times <1micros.

  9. Laser-driven ion acceleration with hollow laser beams

    SciTech Connect

    Brabetz, C. Kester, O.; Busold, S.; Bagnoud, V.; Cowan, T.; Deppert, O.; Jahn, D.; Roth, M.; Schumacher, D.

    2015-01-15

    The laser-driven acceleration of protons from thin foils irradiated by hollow high-intensity laser beams in the regime of target normal sheath acceleration (TNSA) is reported for the first time. The use of hollow beams aims at reducing the initial emission solid angle of the TNSA source, due to a flattening of the electron sheath at the target rear side. The experiments were conducted at the PHELIX laser facility at the GSI Helmholtzzentrum für Schwerionenforschung GmbH with laser intensities in the range from 10{sup 18} W cm{sup −2} to 10{sup 20} W cm{sup −2}. We observed an average reduction of the half opening angle by (3.07±0.42)° or (13.2±2.0)% when the targets have a thickness between 12 μm and 14 μm. In addition, the highest proton energies were achieved with the hollow laser beam in comparison to the typical Gaussian focal spot.

  10. Application of G criterion in metal vapor ion laser

    NASA Astrophysics Data System (ADS)

    Gang, Chen; Bailiang, Pan; Yi, Jin; Kun, Chen; Zhixin, Yao

    2003-09-01

    Application of G criterion to efficient operation of pulsed discharge-excited R-M transition metal vapor laser was successfully extended to univalent ionic lasing medium from neutral atomic lasing medium on the basis of analyzing the simulation results of 1.09 μm Sr + lasing process. All of the known 17 R-M transition laser lines of univalent ions follow the G criterion except one, to which an interpretation is given. Furthermore, we suggest that only 69 lines among 212 possible R-M transition laser lines predicted by S.V. Markova, which satisfy the G criterion, should be explored first.

  11. Production of high-Q ions by laser bombardment method

    SciTech Connect

    Phaneuf, R.A.

    1980-01-01

    The expanding plasma produced when an intense pulse of laser radiation is focused in vacuum onto a solid target has been used as a source of highly stripped ions for collision cross-section measurements. Usable fluxes of carbon nuclei at energies of a few hundred eV/charge have been obtained by irradiation of graphite with pulses of CO/sub 2/ laser radiation at a focused power density of 3 x 10/sup 10/ W/cm/sup 2/. Bombardment of aluminum and iron targets at comparable power levels have yielded ions of maximum charges of 9 and 16, respectively. A time-of-flight apparatus has been constructed to utilize the laser source for measurement of electron capture cross sections for highly stripped ions in gases at energies in the few hundred eV/charge range. Apertures collimate an ion beam from the plasma blowoff, and an electrostatic analyzer selects ions from the expanding plasma which have the same energy per charge. The beam is directed through a gas target cell, charge analyzed once more by deceleration, and detected by a channel plate electron multiplier used in a current amplification mode. Electron capture cross sections have been measured for C/sup +q/ ions, q = 3, 4, 5 in H/sub 2/ at energies ranging from 150 to 1160 eV/charge.

  12. Optimum laser intensity for the production of energetic deuterium ions from laser-cluster interaction

    SciTech Connect

    Bang, W.; Dyer, G.; Quevedo, H. J.; Bernstein, A. C.; Gaul, E.; Rougk, J.; Aymond, F.; Donovan, M. E.; Ditmire, T.

    2013-09-15

    We measured, using Petawatt-level pulses, the average ion energy and neutron yield in high-intensity laser interactions with molecular clusters as a function of laser intensity. The interaction volume over which fusion occurred (1–10 mm{sup 3}) was larger than previous investigations, owing to the high laser power. Possible effects of prepulses were examined by implementing a pair of plasma mirrors. Our results show an optimum laser intensity for the production of energetic deuterium ions both with and without the use of the plasma mirrors. We measured deuterium plasmas with 14 keV average ion energies, which produced 7.2 × 10{sup 6} and 1.6 × 10{sup 7} neutrons in a single shot with and without plasma mirrors, respectively. The measured neutron yields qualitatively matched the expected yields calculated using a cylindrical plasma model.

  13. Accelerated solvent extraction followed by on-line solid-phase extraction coupled to ion trap LC/MS/MS for analysis of benzalkonium chlorides in sediment samples

    USGS Publications Warehouse

    Ferrer, I.; Furlong, E.T.

    2002-01-01

    Benzalkonium chlorides (BACs) were successfully extracted from sediment samples using a new methodology based on accelerated solvent extraction (ASE) followed by an on-line cleanup step. The BACs were detected by liquid chromatography/ion trap mass spectrometry (LC/MS) or tandem mass spectrometry (MS/MS) using an electrospray interface operated in the positive ion mode. This methodology combines the high efficiency of extraction provided by a pressurized fluid and the high sensitivity offered by the ion trap MS/MS. The effects of solvent type and ASE operational variables, such as temperature and pressure, were evaluated. After optimization, a mixture of acetonitrile/water (6:4 or 7:3) was found to be most efficient for extracting BACs from the sediment samples. Extraction recoveries ranged from 95 to 105% for C12 and C14 homologues, respectively. Total method recoveries from fortified sediment samples, using a cleanup step followed by ASE, were 85% for C12BAC and 79% for C14-BAC. The methodology developed in this work provides detection limits in the subnanogram per gram range. Concentrations of BAC homologues ranged from 22 to 206 ??g/kg in sediment samples from different river sites downstream from wastewater treatment plants. The high affinity of BACs for soil suggests that BACs preferentially concentrate in sediment rather than in water.

  14. High-Quality Ion Beam Generation in Laser Plasma Interaction

    NASA Astrophysics Data System (ADS)

    Nagashima, Toshihiro; Takano, Masahiro; Izumiyzma, Takeshi; Barada, Daisuke; Kawata, Shigeo; Gu, Yan Jun; Kong, Qing; Xiao Wang, Ping; Ma, Yan Yun; Wang, Wei Min

    We focus on a control of generation of high-quality ion beam. In this study, near-critical density plasmas are employed and are illuminated by high intensity short laser pulses; we have successfully generated high-energy ions by multiple-stages acceleration. We performed particle-in-cell simulations in this paper. Near-critical density plasmas are employed at the proton source and also in the post acceleration. A beam bunching method is also proposed to control the ion beam length.

  15. Rare earth ion doped non linear laser crystals

    NASA Astrophysics Data System (ADS)

    Jaque, D.; Romero, J. J.; Ramirez, M. O.; Garcia, J. A. S.; de Las Heras, C.; Bausa, L. E.; Sole, J. G.

    2003-01-01

    We show how non linear crystals activated with Yb3+ or Nd3+ ions can be used to develop diode pumped solid state lasers emitting in the visible region of the electromagnetic spectrum. For this purpose we have selected relevant examples of systems investigated in our laboratory.

  16. AISI/DOE Advanced Process Control Program Vol. 4 of 6: ON-LINE, NON-DESTRUCTIVE MECHANICAL PROPERTY MEASUREMENT USING LASER-ULTRASOUND

    SciTech Connect

    Andre' Moreau; Martin Lord; Daniel Levesqure; Marc Dubois; Jean Bussiere; Jean-Pierre Monchalin; Christian Padioleau; Guy Lamouche; Teodor Veres; Martin Viens; Harold Hebert; Pierre Basseras; Cheng-Kuei Jen

    2001-03-31

    The goal of this project was to demonstrate the feasibility to measure the mechanical properties, such as yield strength, tensile strength, elongation, strain hardening exponent and plastic strain ratio parameters, of low carbon steel sheets on the production line using laser ultrasound. The ultrasound generated by the developed apparatus travels mostly back and forth in the thickness of the steel sheet. By measuring the time delay between two echoes, and the relative amplitude of these two echoes, one can measure ultrasound velocity and attenuation. These are governed by the microstructure: grain size, crystallographic texture, dislocations, etc. Thus, by recording the time behavior of the ultrasonic signal, one can extract microstructural information. These microstructural information together with the modified Hall-Petch equation allow measurement of the mechanical properties. Through laboratory investigations with a laboratory laser ultrasound system, followed by the installation of a prototype system at LTV Steel Company's No.1 Inspection Line in Cleveland, all target mechanical properties of ultra low carbon (ULC), low carbon (LC) and high strength low alloy (HSLA) steel sample lots were measured meeting or nearly meeting all the target accuracies. Thus, the project realized its goal to demonstrate that the mechanical properties of low carbon steel sheets can be measured on-line using laser ultrasound

  17. Preliminary result of rapid solenoid for controlling heavy-ion beam parameters of laser ion source

    DOE PAGES

    Okamura, M.; Sekine, M.; Ikeda, S.; Kanesue, T.; Kumaki, M.; Fuwa, Y.

    2015-03-13

    To realize a heavy ion inertial fusion driver, we have studied a possibility of laser ion source (LIS). A LIS can provide high current high brightness heavy ion beams, however it was difficult to manipulate the beam parameters. To overcome the issue, we employed a pulsed solenoid in the plasma drift section and investigated the effect of the solenoid field on singly charged iron beams. The rapid ramping magnetic field could enhance limited time slice of the current and simultaneously the beam emittance changed accordingly. This approach may also useful to realize an ion source for HIF power plant.

  18. Laser stripping of relativistic H{sup {minus}} ions with practical considerations

    SciTech Connect

    Tomlin, R.

    1995-12-01

    This paper describes laser stripping of H{sup {minus}} ions. Some applications are suggested for HEP including stripping 2GeV ions circulating in an accelerator with radius 75 meters where laser meets ion head on in a three meter interaction region. The paper describes photoionizaton cross section, laser power calculation, and how to generate the 5 micrometer light.

  19. Selective deuterium ion acceleration using the Vulcan petawatt laser

    SciTech Connect

    Krygier, A. G.; Morrison, J. T.; Kar, S. Ahmed, H.; Alejo, A.; Green, A.; Jung, D.; Clarke, R.; Notley, M.; Fuchs, J.; Vassura, L.; Kleinschmidt, A.; Roth, M.; Najmudin, Z.; Nakamura, H.; Norreys, P.; Oliver, M.; Zepf, M.; Borghesi, M.; Freeman, R. R.

    2015-05-15

    We report on the successful demonstration of selective acceleration of deuterium ions by target-normal sheath acceleration (TNSA) with a high-energy petawatt laser. TNSA typically produces a multi-species ion beam that originates from the intrinsic hydrocarbon and water vapor contaminants on the target surface. Using the method first developed by Morrison et al. [Phys. Plasmas 19, 030707 (2012)], an ion beam with >99% deuterium ions and peak energy 14 MeV/nucleon is produced with a 200 J, 700 fs, >10{sup 20}W/cm{sup 2} laser pulse by cryogenically freezing heavy water (D{sub 2}O) vapor onto the rear surface of the target prior to the shot. Within the range of our detectors (0°–8.5°), we find laser-to-deuterium-ion energy conversion efficiency of 4.3% above 0.7 MeV/nucleon while a conservative estimate of the total beam gives a conversion efficiency of 9.4%.

  20. Saturation of multi-laser beams laser-plasma instabilities from stochastic ion heating

    SciTech Connect

    Michel, P.; Williams, E. A.; Divol, L.; Berger, R. L.; Glenzer, S. H.; Callahan, D. A.; Rozmus, W.

    2013-05-15

    Cross-beam energy transfer (CBET) has been used as a tool on the National Ignition Facility (NIF) since the first energetics experiments in 2009 to control the energy deposition in ignition hohlraums and tune the implosion symmetry. As large amounts of power are transferred between laser beams at the entrance holes of NIF hohlraums, the presence of many overlapping beat waves can lead to stochastic ion heating in the regions where laser beams overlap [P. Michel et al., Phys. Rev. Lett. 109, 195004 (2012)]. This increases the ion acoustic velocity and modifies the ion acoustic waves’ dispersion relation, thus reducing the plasma response to the beat waves and the efficiency of CBET. This pushes the plasma oscillations driven by CBET in a regime where the phase velocities are much smaller than both the electron and ion thermal velocities. CBET gains are derived for this new regime and generalized to the case of multi ion species plasmas.

  1. Pulsed hollow-cathode ion lasers: pumping and lasing parameters

    SciTech Connect

    Zinchenko, S P; Ivanov, I G

    2012-06-30

    Optimal discharge conditions have been experimentally found for ion lasers excited in the hollow-cathode discharge plasma by microsecond current pulses by pumping working atoms in secondkind collisions with ions and metastable buffer-gas atoms. Measurements of the output power of krypton ion and zinc-, cadmium-, mercury-, thallium-, copper-, and gallium-vapour lasers in tubes with cathodes of different diameters showed that the pulse power reaches several tens of watts, and the average power obtained with cathodes 2 cm in diameter and a length of 40 cm or more approaches 1 W. Lasing in most media is observed simultaneously at several lines (the multi-wavelength regime). Lasing on a three-component (He - Kr - Hg) mixture is realised in the multi-wavelength regime at blue, red, and IR lines.

  2. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited).

    PubMed

    Zhao, H Y; Zhang, J J; Jin, Q Y; Liu, W; Wang, G C; Sun, L T; Zhang, X Z; Zhao, H W

    2016-02-01

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 10(13) W cm(-2) in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications.

  3. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited)

    NASA Astrophysics Data System (ADS)

    Zhao, H. Y.; Zhang, J. J.; Jin, Q. Y.; Liu, W.; Wang, G. C.; Sun, L. T.; Zhang, X. Z.; Zhao, H. W.

    2016-02-01

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 1013 W cm-2 in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications.

  4. New development of laser ion source for highly charged ion beam production at Institute of Modern Physics (invited).

    PubMed

    Zhao, H Y; Zhang, J J; Jin, Q Y; Liu, W; Wang, G C; Sun, L T; Zhang, X Z; Zhao, H W

    2016-02-01

    A laser ion source based on Nd:YAG laser has been being studied at the Institute of Modern Physics for the production of high intensity high charge state heavy ion beams in the past ten years, for possible applications both in a future accelerator complex and in heavy ion cancer therapy facilities. Based on the previous results for the production of multiple-charged ions from a wide range of heavy elements with a 3 J/8 ns Nd:YAG laser [Zhao et al., Rev. Sci. Instrum. 85, 02B910 (2014)], higher laser energy and intensity in the focal spot are necessary for the production of highly charged ions from the elements heavier than aluminum. Therefore, the laser ion source was upgraded with a new Nd:YAG laser, the maximum energy of which is 8 J and the pulse duration can be adjusted from 8 to 18 ns. Since then, the charge state distributions of ions from various elements generated by the 8 J Nd:YAG laser were investigated for different experimental conditions, such as laser energy, pulse duration, power density in the focal spot, and incidence angle. It was shown that the incidence angle is one of the most important parameters for the production of highly charged ions. The capability of producing highly charged ions from the elements lighter than silver was demonstrated with the incidence angle of 10° and laser power density of 8 × 10(13) W cm(-2) in the focal spot, which makes a laser ion source complementary to the superconducting electron cyclotron resonance ion source for the future accelerator complex especially in terms of the ion beam production from some refractory elements. Nevertheless, great efforts with regard to the extraction of intense ion beams, modification of the ion beam pulse duration, and reliability of the ion source still need to be made for practical applications. PMID:26931978

  5. Detection and quantification of sulfur in oil products by laser-induced breakdown spectroscopy for on-line analysis

    NASA Astrophysics Data System (ADS)

    Trichard, F.; Forquet, V.; Gilon, N.; Lienemann, C.-P.; Baco-Antoniali, F.

    2016-04-01

    Determination of sulfur in petroleum products is described using Laser Induced breakdown spectroscopy (LIBS). A study of buffer gases employed to improve sulfur IR line detection is presented. Optimisation of the flow rate led to a 1.4 L/min optimal helium flow rate. An adaptation between a typical laboratory setup to a compact system allowed to obtain detection limits in the 0.2% w/w range. Calibration is made under the process conditions (70 °C) and at room temperature. Normalization with a helium emission line compensates for liquid level variations and for the temperature variations. The analysis of a sample over the course of 2 days under the conditions of the industrial process was tested and gave a good repeatability.

  6. Means and method for characterizing high power, ultra short laser pulses in a real time, on line manner

    DOEpatents

    Veligdan, James T.

    1994-01-01

    An ultra short (<10 ps), high power laser pulse is temporally characterized by a system that uses a physical measurement of a wavefront that has been altered in a known manner. The system includes a first reflection switch to remove a portion of a pulse from a beam of pulses, then includes a second reflection switch, operating in a mode that is opposite to the first reflection switch, to slice off a portion of that removed portion. The sliced portion is then directed to a measuring device for physical measurement. The two reflection switches are arranged with respect to each other and with respect to the beam of ultra short pulses such that physical measurement of the sliced portion is related to the temporal measurement of the ultra short pulse by a geometric or trigonometric relationship. The reflection switches are operated by a control pulse that is directed to impinge on each of the reflection switches at a 90.degree. angle of incidence.

  7. Amplitude Noise Reduction of Ion Lasers with Optical Feedback

    NASA Technical Reports Server (NTRS)

    Herring, Gregory C.

    2011-01-01

    A reduction in amplitude noise on the output of a multi-mode continuous-wave Ar-ion laser was previously demonstrated when a fraction of the output power was retroreflected back into the laser cavity. This result was reproduced in the present work and a Fabry-Perot etalon was used to monitor the longitudinal mode structure of the laser. A decrease in the number of operating longitudinal cavity modes was observed simultaneously with the introduction of the optical feedback and the onset of the amplitude noise reduction. The noise reduction is a result of a reduced number of lasing modes, resulting in less mode beating and amplitude fluctuations of the laser output power.

  8. Negative ion beam generation in laser plasma interactions

    NASA Astrophysics Data System (ADS)

    Jequier, Sophie; Tikhonchuk, Vladimir; Ter-Avetisyan, Sargis

    2013-10-01

    Detection of a large number of energetic negative ions and neutral atoms have been reported in recent intense laser plasma interaction experiments. These particles were produced from fast positive ions (proton, carbon, oxygen) accelerated from a laser produced plasma when they were passing through a cold spray of water or ethanol. The negative ions formation is strongly related to the fast positive ions, and it is explained by a process of a single electron capture - loss. Double charge exchange, elastic scattering and energy loss phenomena have been neglected since their cross sections are much smaller. Assuming independent atoms approximation, we study populations evolution through the interaction zone analytically and numerically by solving the rate equations using cross sections drawn from literature. Taking into account the energy distribution of the incident ions, the calculations give the final energy distribution for the different species that can be compared to experimental spectra. First results obtained for hydrogen in the water case indicate that this model can explain the main observed features. The results concerning the carbon and oxygen ions will be also presented as well as refinement of the cross sections since some cross sections are missing for these energies.

  9. New on-line method for water isotope analysis of speleothem fluid inclusions using laser absorption spectroscopy (WS-CRDS)

    NASA Astrophysics Data System (ADS)

    Affolter, S.; Fleitmann, D.; Leuenberger, M.

    2014-01-01

    A new online method to analyse water isotopes of speleothem fluid inclusions using a wavelength scanned cavity ring down spectroscopy (WS-CRDS) instrument is presented. This novel technique allows us to simultaneously measure hydrogen and oxygen isotopes for a released aliquot of water. To do so, we designed a new simple line that allows the on-line water extraction and isotope analysis of speleothem samples. The specificity of the method lies in the fact that fluid inclusions release is made on a standard water background, which mainly improves the δD reliability. To saturate the line, a peristaltic pump continuously injects standard water into the line that is permanently heated to 140 °C and flushed with dry nitrogen gas. This permits instantaneous and complete vaporisation of the standard water resulting in an artificial water background with well-known δD and δ18O values. The speleothem sample is placed into a copper tube, attached to the line and after system stabilisation is crushed using a simple hydraulic device to liberate speleothem fluid inclusions water. The released water is carried by the nitrogen/standard water gas stream directly to a Picarro L1102-i for isotope determination. To test the accuracy and reproducibility of the line and to measure standard water during speleothem measurements a syringe injection unit was added to the line. Peak evaluation is done similarly as in gas chromatography to obtain δD and δ18O isotopic composition of measured water aliquots. Precision is better than 1.5‰ for δD and 0.4‰ for δ18O for water measurement for an extended range (-210 to 0‰ for δD and -27 to 0‰ for δ18O) primarily dependent on the amount of water released from speleothem fluid inclusions and secondarily on the isotopic composition of the sample. The results show that WS-CRDS technology is suitable for speleothem fluid inclusion measurements and gives results that are comparable to Isotope Ratio Mass Spectrometry (IRMS) technique.

  10. Ion-beam assisted laser fabrication of sensing plasmonic nanostructures

    PubMed Central

    Kuchmizhak, Aleksandr; Gurbatov, Stanislav; Vitrik, Oleg; Kulchin, Yuri; Milichko, Valentin; Makarov, Sergey; Kudryashov, Sergey

    2016-01-01

    Simple high-performance, two-stage hybrid technique was developed for fabrication of different plasmonic nanostructures, including nanorods, nanorings, as well as more complex structures on glass substrates. In this technique, a thin noble-metal film on a dielectric substrate is irradiated by a single tightly focused nanosecond laser pulse and then the modified region is slowly polished by an accelerated argon ion (Ar+) beam. As a result, each nanosecond laser pulse locally modifies the initial metal film through initiation of fast melting and subsequent hydrodynamic processes, while the following Ar+-ion polishing removes the rest of the film, revealing the hidden topography features and fabricating separate plasmonic structures on the glass substrate. We demonstrate that the shape and lateral size of the resulting functional plasmonic nanostructures depend on the laser pulse energy and metal film thickness, while subsequent Ar+-ion polishing enables to vary height of the resulting nanostructures. Plasmonic properties of the fabricated nanostructures were characterized by dark-field micro-spectroscopy, Raman and photoluminescence measurements performed on single nanofeatures, as well as by supporting numerical calculations of the related electromagnetic near-fields and Purcell factors. The developed simple two-stage technique represents a new step towards direct large-scale laser-induced fabrication of highly ordered arrays of complex plasmonic nanostructures. PMID:26776569

  11. Intense Laser Ionization and Acceleration of Electrons in Highly-Charged Ions Using Vortex Laser Beams

    NASA Astrophysics Data System (ADS)

    Pi, Liang-Wen; Vikartofsky, Andrew; Starace, Anthony F.

    2016-05-01

    Recent advances in laser technology have led to the development of high-power petawatt lasers, making possible laser intensities of the order of 1022 W /cm2 . An electron in a highly-charged ion can be ionized in a laser field at its peak intensity and swiftly accelerated to GeV energies. Our prior investigation of laser acceleration of electrons using linearly-polarized Gaussian beams (with zero orbital angular momentum) has revealed that the final-state energies and ejection angles of the electrons depend on the initial target ion positions relative to the laser focus. We report here recent simulations of laser ionization and acceleration of electrons using linearly-polarized vortex laser beams (i.e., Laguerre-Gaussian beams), which carry orbital angular momentum and can spin microscopic objects. These simulations show that the inherent spiral phase structure of the vortex beams leads to improved final-state energy and ejection angle distributions of the electrons. This work is supported in part by DOE, Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences, under Grant No. DE-FG02-96ER14646.

  12. Means and method for characterizing high power, ultra short laser pulses in a real time, on line manner

    DOEpatents

    Veligdan, J.T.

    1994-03-08

    An ultra short (<10 ps), high power laser pulse is temporally characterized by a system that uses a physical measurement of a wavefront that has been altered in a known manner. The system includes a first reflection switch to remove a portion of a pulse from a beam of pulses, then includes a second reflection switch, operating in a mode that is opposite to the first reflection switch, to slice off a portion of that removed portion. The sliced portion is then directed to a measuring device for physical measurement. The two reflection switches are arranged with respect to each other and with respect to the beam of ultra short pulses such that physical measurement of the sliced portion is related to the temporal measurement of the ultra short pulse by a geometric or trigonometric relationship. The reflection switches are operated by a control pulse that is directed to impinge on each of the reflection switches at a 90[degree] angle of incidence. 8 figures.

  13. Simultaneous and sensitive analysis of aliphatic carboxylic acids by ion-chromatography using on-line complexation with copper(II) ion.

    PubMed

    Kemmei, Tomoko; Kodama, Shuji; Yamamoto, Atsushi; Inoue, Yoshinori; Hayakawa, Kazuichi

    2015-01-01

    A new approach to ion chromatography is proposed to improve the UV detection of aliphatic carboxylic acids separated by anion-exchange chromatography. When copper(II) ion added to the mobile phase, it forms complexes with carboxylic acids that can be detected at 240 nm. The absorbance was found to increase with increasing copper(II) ion concentration. The retention times of α-hydroxy acids were also found to depend on the copper(II) ion concentration. Addition of acetonitrile to the mobile phase improved the separation of aliphatic carboxylic acids. The detection limits of the examined carboxylic acids (formate, glycolate, acetate, lactate, propionate, 3-hydroxypropionate, n-butyrate, isobutyrate, n-valerate, isovalerate, n-caproate) calculated at S/N=3 ranged from 0.06 to 3 μM. The detector signal was linear over three orders of magnitude of carboxylic acid concentration. The proposed method was successfully applied to analyze aliphatic carboxylic acids in rainwater and bread.

  14. On-line quality assurance of rotational radiotherapy treatment delivery by means of a 2D ion chamber array and the Octavius phantom

    SciTech Connect

    Esch, Ann van; Clermont, Christian; Devillers, Magali; Iori, Mauro; Huyskens, Dominique P.

    2007-10-15

    For routine pretreatment verification of innovative treatment techniques such as (intensity modulated) dynamic arc therapy and helical TomoTherapy, an on-line and reliable method would be highly desirable. The present solution proposed by TomoTherapy, Inc. (Madison, WI) relies on film dosimetry in combination with up to two simultaneous ion chamber point dose measurements. A new method is proposed using a 2D ion chamber array (Seven29, PTW, Freiburg, Germany) inserted in a dedicated octagonal phantom, called Octavius. The octagonal shape allows easy positioning for measurements in multiple planes. The directional dependence of the response of the detector was primarily investigated on a dual energy (6 and 18 MV) Clinac 21EX (Varian Medical Systems, Palo Alto, CA) as no fixed angle incidences can be calculated in the Hi-Art TPS of TomoTherapy. The array was irradiated from different gantry angles and with different arc deliveries, and the dose distributions at the level of the detector were calculated with the AAA (Analytical Anisotropic Algorithm) photon dose calculation algorithm implemented in Eclipse (Varian). For validation on the 6 MV TomoTherapy unit, rotational treatments were generated, and dose distributions were calculated with the Hi-Art TPS. Multiple cylindrical ion chamber measurements were used to cross-check the dose calculation and dose delivery in Octavius in the absence of the 2D array. To compensate for the directional dependence of the 2D array, additional prototypes of Octavius were manufactured with built-in cylindrically symmetric compensation cavities. When using the Octavius phantom with a 2 cm compensation cavity, measurements with an accuracy comparable to that of single ion chambers can be achieved. The complete Octavius solution for quality assurance of rotational treatments consists of: The 2D array, two octagonal phantoms (with and without compensation layer), an insert for nine cylindrical ion chambers, and a set of inserts of

  15. Negative Ion Detection Using Laser Thomson Scattering Combined with Laser Photodetachment

    NASA Astrophysics Data System (ADS)

    Kono, A.; Ohno, J.; Funahashi, H.

    2001-10-01

    A purely optical technique for detecting negative ions in plasmas has been demonstrated where laser-photodetached electrons are detected via laser Thomson scattering. The technique allows one to obtain high spatial resolution (difficult to obtain using microwave techniques) without using a Langmuir probe. The plasma was irradiated by frequency-quadrupled (266nm) and frequency-doubled (532 nm) Nd:YAG laser beams originating from the same laser oscillator; the 266 nm beam causes photodetachment, while the 532 nm beam serves as the light source for Thomson scattering. It was so arranged that the 266 nm laser pulse irradiates the plasma 10 ns (>laser pulse width) earlier than the 532 nm laser pulse and, in the observation region, the focused thin 532 nm beam forms the coaxial core of the unfocused 266 nm beam. A specially designed triple-grating spectrometer was used, which produces Thomson spectra on the output focal plane with the interfering Rayleigh and stray components highly suppressed; an ICCD camera operated in the photon-counting mode was used for multichannel detection of the spectrum. Measurements for inductively coupled NF_3(5%)/Ar and SF_6(5%)/Ar plasmas at 25 mTorr with electron densities of ~ 10^11 cm-3 indicated that the negative ion density is of comparable magnitude to the electron density.

  16. An inductively heated hot cavity catcher laser ion source

    SciTech Connect

    Reponen, M.; Moore, I. D. Pohjalainen, I.; Savonen, M.; Voss, A.; Rothe, S.; Sonnenschein, V.

    2015-12-15

    An inductively heated hot cavity catcher has been constructed for the production of low-energy ion beams of exotic, neutron-deficient Ag isotopes. A proof-of-principle experiment has been realized by implanting primary {sup 107}Ag{sup 21+} ions from a heavy-ion cyclotron into a graphite catcher. A variable-thickness nickel foil was used to degrade the energy of the primary beam in order to mimic the implantation depth expected from the heavy-ion fusion-evaporation recoils of N = Z {sup 94}Ag. Following implantation, the silver atoms diffused out of the graphite and effused into the catcher cavity and transfer tube, where they were resonantly laser ionized using a three-step excitation and ionization scheme. Following mass separation, the ions were identified by scanning the frequency of the first resonant excitation step while recording the ion count rate. Ion release time profiles were measured for different implantation depths and cavity temperatures with the mean delay time varying from 10 to 600 ms. In addition, the diffusion coefficients for silver in graphite were measured for temperatures of 1470 K, 1630 K, and 1720 K, from which an activation energy of 3.2 ± 0.3 eV could be determined.

  17. An inductively heated hot cavity catcher laser ion source.

    PubMed

    Reponen, M; Moore, I D; Pohjalainen, I; Rothe, S; Savonen, M; Sonnenschein, V; Voss, A

    2015-12-01

    An inductively heated hot cavity catcher has been constructed for the production of low-energy ion beams of exotic, neutron-deficient Ag isotopes. A proof-of-principle experiment has been realized by implanting primary (107)Ag(21+) ions from a heavy-ion cyclotron into a graphite catcher. A variable-thickness nickel foil was used to degrade the energy of the primary beam in order to mimic the implantation depth expected from the heavy-ion fusion-evaporation recoils of N = Z (94)Ag. Following implantation, the silver atoms diffused out of the graphite and effused into the catcher cavity and transfer tube, where they were resonantly laser ionized using a three-step excitation and ionization scheme. Following mass separation, the ions were identified by scanning the frequency of the first resonant excitation step while recording the ion count rate. Ion release time profiles were measured for different implantation depths and cavity temperatures with the mean delay time varying from 10 to 600 ms. In addition, the diffusion coefficients for silver in graphite were measured for temperatures of 1470 K, 1630 K, and 1720 K, from which an activation energy of 3.2 ± 0.3 eV could be determined. PMID:26724021

  18. An inductively heated hot cavity catcher laser ion source

    NASA Astrophysics Data System (ADS)

    Reponen, M.; Moore, I. D.; Pohjalainen, I.; Rothe, S.; Savonen, M.; Sonnenschein, V.; Voss, A.

    2015-12-01

    An inductively heated hot cavity catcher has been constructed for the production of low-energy ion beams of exotic, neutron-deficient Ag isotopes. A proof-of-principle experiment has been realized by implanting primary 107Ag21+ ions from a heavy-ion cyclotron into a graphite catcher. A variable-thickness nickel foil was used to degrade the energy of the primary beam in order to mimic the implantation depth expected from the heavy-ion fusion-evaporation recoils of N = Z 94Ag. Following implantation, the silver atoms diffused out of the graphite and effused into the catcher cavity and transfer tube, where they were resonantly laser ionized using a three-step excitation and ionization scheme. Following mass separation, the ions were identified by scanning the frequency of the first resonant excitation step while recording the ion count rate. Ion release time profiles were measured for different implantation depths and cavity temperatures with the mean delay time varying from 10 to 600 ms. In addition, the diffusion coefficients for silver in graphite were measured for temperatures of 1470 K, 1630 K, and 1720 K, from which an activation energy of 3.2 ± 0.3 eV could be determined.

  19. VUV (vacuum ultraviolet) laser diagnostics of H sup - ion sources

    SciTech Connect

    Young, A.T.; Stutzin, G.C.; Leung, K.N.; Kunkel, W.B.

    1989-11-01

    Vacuum ultraviolet laser absorption spectroscopy has been employed to measure the populations and temperatures of ground electronic state H-atoms and vibrationally-excited H{sub 2} molecules in a volume H{sup -} ion source. Measurements of both species have been made under a variety of discharge conditions. Vibrational levels to v{double prime}=8 have been measured, with the vibrational population distribution well described by a temperature of 4150K. 10 refs., 9 figs.

  20. Laser and focused ion beam combined machining for micro dies.

    PubMed

    Yoshida, Y; Okazaki, W; Uchida, T

    2012-02-01

    We have developed a laser and focused ion beam (FIB) compound process for press mold dies of a micro lens array (MLA) and a micro needle array (MNA) in a glassy carbon (GC). The press mold die of the MLA was roughly fabricated by UV-YAG laser. After this process, we finished this surface by scanning FIB. As a result, higher accuracy and good roughness of surface profile can be realized. An optical glass is used to confirm the shape of lens. Moreover, we fabricated 6 × 6 through-holes in the GC by the spiral drilling in addition to the focus position movement of the UV laser for press mold die of the MNA. After the FIB process, we were able to make the needle die of surface and hole wall roughness less than 0.9 μm. A silicon rubber is used to confirm the shape of the holes.

  1. Ion acceleration using high-contrast ultra-intense lasers

    NASA Astrophysics Data System (ADS)

    Fuchs, J.; Antici, P.; D'Humières, E.; Lefebvre, E.; Borghesi, M.; Brambrink, E.; Cecchetti, C.; Toncian, T.; Pépin, H.; Audebert, P.

    2006-06-01

    We have compared the acceleration of high-energy ions from the rear-surface of thin foils for various contrast conditions of the ultra-intense laser pulse irradiating the targets. The experiments were performed using the LULI 100 TW facility. We used Al targets of variable thicknesses and the laser pulse contrast ratio ahead of the main pulse was varied using either a fast Pockels cell or a single or double plasma mirror. The latter was installed at an intermediate field position, in between the focusing optics and the target, so that its effect was optimized. By improving with these two methods the laser pulse contrast, we have observed that we could significantly reduce the thickness of the target used for proton acceleration and at the same time increase both the cut-off energy of the accelerated protons and the energy conversion efficiency of the process.

  2. Laser acceleration of low emittance, high energy ions and applications

    NASA Astrophysics Data System (ADS)

    Fuchs, Julien; Audebert, Patrick; Borghesi, Marco; Pépin, Henri; Willi, Oswald

    2009-03-01

    Laser-accelerated ion sources have exceptional properties, i.e. high brightness and high spectral cut-off (56 MeV at present), high directionality and laminarity (at least 100-fold better than conventional accelerators beams), short burst duration (ps). Thanks to these properties, these sources open new opportunities for applications. Among these, we have already explored their use for proton radiography of fields in plasmas and for warm dense matter generation. These sources could also stimulate development of compact ion accelerators or be used for medical applications. To extend the range of applications, ion energy and conversion efficiency must however be increased. Two strategies for doing so using present-day lasers have been successfully explored in LULI experiments. In view of applications, it is also essential to control (i.e. collimate and energy select) these beams. For this purpose, we have developed an ultra-fast laser-triggered micro-lens providing tuneable control of the beam divergence as well as energy selection. To cite this article: J. Fuchs et al., C. R. Physique 10 (2009).

  3. Low charge state heavy ion production with sub-nanosecond laser.

    PubMed

    Kanesue, T; Kumaki, M; Ikeda, S; Okamura, M

    2016-02-01

    We have investigated laser ablation plasma of various species using nanosecond and sub-nanosecond lasers for both high and low charge state ion productions. We found that with sub-nanosecond laser, the generated plasma has a long tail which has low charge state ions determined by an electrostatic ion analyzer even under the laser irradiation condition for highly charged ion production. This can be caused by insufficient laser absorption in plasma plume. This property might be suitable for low charge state ion production. We used a nanosecond laser and a sub-nanosecond laser for low charge state ion production to investigate the difference of generated plasma using the Zirconium target. PMID:26931977

  4. Relative ion expansion velocity in laser-produced plasmas

    NASA Technical Reports Server (NTRS)

    Goldsmith, S.; Moreno, J. C.; Griem, H. R.; Cohen, Leonard; Richardson, M. C.

    1988-01-01

    The spectra of highly ionized titanium, Ti XIII through Ti XXI, and C VI Lyman lines were excited in laser-produced plasmas. The plasma was produced by uniformly irradiating spherical glass microballoons coated with thin layers of titanium and parylene. The 24-beam Omega laser system produced short, 0.6 ns, and high-intensity, 4 x 10 to the 14th W/sq cm, laser pulses at a wavelength of 351 nm. The measured wavelength for the 2p-3s Ti XIII resonance lines had an average shift of + 0.023 A relative to the C VI and Ti XX spectral lines. No shift was found between the C VI, Ti XIX, and Ti XX lines. The shift is attributed to a Doppler effect, resulting from a difference of (2.6 + or - 0.2) x 10 to the 7th cm/s in the expansion velocities of Ti XIX and Ti XX ions compared to Ti XIII ions.

  5. Beam Extraction from Laser Driven Multi-Charged Ion Source

    SciTech Connect

    Anderson, O A; Logan, B G

    2001-03-19

    A newly proposed type of multicharged ion source offers the possibility of an economically advantageous high-charge-state fusion driver. Multiphoton absorption in an intense uniform laser focus can give multiple charge states of high purity, simplifying or eliminating the need for charge-state separation downstream. Very large currents (hundreds of amperes) can be extracted from this type of source. Several arrangements are possible. For example, the laser plasma could be tailored for storage in a magnetic bucket, with beam extracted from the bucket. A different approach, described in this report, is direct beam extraction from the expanding laser plasma. They discuss extraction and focusing for the particular case of a 4.1-MV beam of Xe{sup 16+} ions. The maximum duration of the beam pulse is limited by the total charge in the plasma, while the practical pulse length is determined by the range of plasma radii over which good beam optics can be achieved. The extraction electrode contains a solenoid for beam focusing. The design studies were carried out first with an envelope code and then with a self-consistent particle code. Results from the initial model showed that hundreds of amperes could be extracted, but that most of this current missed the solenoid entrance or was intercepted by the wall and that only a few amperes were able to pass through. They conclude with an improved design which increases the surviving beam to more than 70 amperes.

  6. Development of a Versatile Laser Ultrasonic System and Application to On-Line Measurement for Process Control of Wall Thickness and Eccentrictiy of Steel Seamless Mechanical Tubing

    SciTech Connect

    Kisner, R.A.; Kercel, S.W.; Damiano, B.; Bingham, P.R.; Gee, T.F.; Tucker, R.W.; Moore, M.R.; Hileman, M.; Emery, M.; Lenarduzzi, R.; Hardy, J.E.; Weaver, K.; Crutcher, R.; Kolarik, R.V., II; Vandervaart, R.H.

    2002-04-24

    Researchers at the Timken Company conceived a project to develop an on-line instrument for wall thickness measurement of steel seamless mechanical tubing based on laser ultrasonic technology. The instrument, which has been installed and tested at a piercing mill, provides data on tube eccentricity and concentricity. Such measurements permit fine-tuning of manufacturing processes to eliminate excess material in the tube wall and therefore provide a more precisely dimensioned product for their customers. The resulting process energy savings are substantial, as is lowered environmental burden. The expected savings are $85.8 million per year in seamless mechanical tube piercing alone. Applied across the industry, this measurement has a potential of reducing energy consumption by 6 x 10{sup 12} BTU per year, greenhouse gas emissions by 0.3 million metric tons carbon equivalent per year, and toxic waste by 0.255 million pounds per year. The principal technical contributors to the project were the Timken Company, Industrial Materials Institute (IMI, a contractor to Timken), and Oak Ridge National Laboratory (ORNL). Timken provided mill access as well as process and metallurgical understanding. Timken researchers had previously developed fundamental ultrasonic analysis methods on which this project is based. IMI developed and fabricated the laser ultrasonic generation and receiver systems. ORNL developed Bayesian and wavelet based real-time signal processing, spread-spectrum wireless communication, and explored feature extraction and pattern recognition methods. The resulting instrument has successfully measured production tubes at one of Timken's piercing mills. This report concentrates on ORNL's contribution through the CRADA mechanism. The three components of ORNL's contribution were met with mixed success. The real-time signal-processing task accomplished its goal of improvement in detecting time of flight information with a minimum of false data. The signal processing

  7. Development of laser-ion beam photodissociation methods. Progress report, December 1, 1992--November 30, 1993

    SciTech Connect

    Russell, D.H.

    1992-08-01

    Research efforts were concentrated on developing the tandem magnetic sector (EB)/reflection-time-of-flight (TOF) instrument, preliminary experiments with tandem TOF/TOF instruments, developing method for performing photodissociation with pulsed lasers, experiments with laser ionization of aerosol particles, matrix-assisted laser desorption ionization (MALDI), and ion-molecule reaction chemistry of ground and excited state transition metal ions. This progress report is divided into: photodissociation, MALDI (including aerosols), and ion chemistry fundamentals.

  8. Proposal for laser cooling of rare-earth ions

    NASA Astrophysics Data System (ADS)

    Dulieu, Olivier; Hong, Ye; Wyart, Jean-François; Lepers, Maxence

    2016-05-01

    The efficiency of laser cooling relies on the existence of an almost closed optical-transition cycle in the energy spectrum of the considered species. In this respect, rare-earth elements exhibit many transitions which are likely to induce noticeable leaks from the cooling cycle. In this work, to determine whether laser cooling of singly ionized erbium Er+ is feasible, we have performed accurate electronic-structure calculations of energies and spontaneous-emission Einstein coefficients of Er+, using a combination of ab initio and least-squares-fitting techniques. We identify five weak closed transitions suitable for laser cooling, the broadest of which is in the kilohertz range. For the strongest transitions, by simulating the cascade dynamics of spontaneous emission, we show that repumping is necessary, and we discuss possible repumping schemes.We expect our detailed study on Er+ to give good insight into the laser cooling of neighboring ions such as Dy+. Supported by ``Agence Nationale de la Recherche'' (ANR), under the project COPOMOL (Contract No. ANR-13-IS04-0004-01).

  9. High-Resolution Laser Spectroscopy on the Negative Osmium Ion

    SciTech Connect

    Warring, U.; Amoretti, M.; Canali, C.; Fischer, A.; Heyne, R.; Meier, J. O.; Morhard, Ch.; Kellerbauer, A.

    2009-01-30

    We have applied a combination of laser excitation and electric-field detachment to negative atomic ions for the first time, resulting in an enhancement of the excited-state detection efficiency for spectroscopy by at least 2 orders of magnitude. Applying the new method, a measurement of the bound-bound electric-dipole transition frequency in {sup 192}Os{sup -} was performed using collinear spectroscopy with a narrow-bandwidth cw laser. The transition frequency was found to be 257.831 190(35) THz [wavelength 1162.747 06(16) nm, wave number 8600.3227(12) cm{sup -1}], in agreement with the only prior measurement, but with more than 100-fold higher precision.

  10. Tailored surface modification by ion implantation and laser treatment

    NASA Astrophysics Data System (ADS)

    Picraux, S. T.; Pope, L. E.

    1984-11-01

    Techniques and applications of ion- and laser-beam treatment of surface and near surface materials to control the composition and microstructure are explored. The processes are especially useful in miniaturized electronic components with large surface/volume ratios. Laser beams permit selective, extremely short interval high energy heating of specific molecules in surfaces and studies of transient and metastable states that are otherwise unattainable. The applications affect the wear, friction, hardness, adhesion, fatigue, toughness, ductility, corrosion resistance, and electromagnetic properties of the materials. Beam treatments have been successfully applied to polymers, ceramics, metals, and microprocessors, often causing new performance characteristics to appear. The techniques are noted to relax the usual constraints of thermal equilibrium and thereby increase the understanding of materials.

  11. Simultaneous ion beam profile scan using a single laser source

    NASA Astrophysics Data System (ADS)

    Liu, Y.; Long, C.; Huang, C.; Dickson, R.; Aleksandrov, A.

    2013-01-01

    We report on the world’s first experiment of a simultaneous profile scan of the hydrogen ion (H-) beam using a laser wire system. The system was developed and brought to operational level of application at the superconducting linac of the Spallation Neutron Source accelerator complex. The laser wire profile scanner is based on a photodetachment process and therefore can be conducted on a 1-MW neutron production H- beam in a nonintrusive manner. The new simultaneous profile scanning system allows one to simultaneously measure profiles of the H- beam at nine different locations of the linac with high speed and accuracy, and therefore provides a unique tool for accelerator tuning and physics study. This paper describes the design, optical system and software platform developments, and measurement results of the simultaneous profile scanning system.

  12. Optimal ion acceleration from ultrathin foils irradiated by a profiled laser pulse of relativistic intensity

    SciTech Connect

    Andreev, A. A.; Steinke, S.; Sokollik, T.; Schnuerer, M.; Nickles, P. V.; Avetsiyan, S. Ter; Platonov, K. Yu.

    2009-01-15

    Recent investigations of relativistic laser plasmas have shown that the energy transfer from the laser field to the kinetic ion energy and therefore the attainable maximum energy of the ions increases when ultrathin targets are irradiated by laser pulse without prepulse. In this paper, the influence of the target thickness and laser pulse contrast on the energy of the accelerated ions has been studied theoretically as well as experimentally. An optimum target was searched if a real laser pulse with a certain prepulse irradiates the target.

  13. Ion acceleration and D-D nuclear fusion in laser-generated plasma from advanced deuterated polyethylene.

    PubMed

    Torrisi, Lorenzo

    2014-10-23

    Deuterated polyethylene targets have been irradiated by means of a 1016 W/cm2 laser using 600 J pulse energy, 1315 nm wavelength, 300 ps pulse duration and 70 micron spot diameter. The plasma parameters were measured using on-line diagnostics based on ion collectors, SiC detectors and plastic scintillators, all employed in time-of-flight configuration. In addition, a Thomson parabola spectrometer, an X-ray streak camera, and calibrated neutron dosimeter bubble detectors were employed. Characteristic protons and neutrons at maximum energies of 3.0 MeV and 2.45 MeV, respectively, were detected, confirming that energy spectra of reaction products coming from deuterium-deuterium nuclear fusion occur. In thick advanced targets a fusion rate of the order of 2 × 108 fusions per laser shot was calculated.

  14. Conceptional design of the laser ion source based hadrontherapy facility

    NASA Astrophysics Data System (ADS)

    Xie, Xiu-Cui; Song, Ming-Tao; Zhang, Xiao-Hu

    2014-04-01

    A laser ion source (LIS), which can provide a carbon beam with highly stripped state (C6+) and high intensity (several tens mA), would significantly change the overall design of the hadrontherapy facility. The proposed LIS based hadrontherapy facility has the advantages of short linac length, simple injection scheme, and small synchrotron size. With the experience from the DPIS and HITFiL projects that have been conducted in IMP, a conceptional design of the LIS based hadrontherapy facility will be presented, with special attention given to APF type IH DTL design and simulation.

  15. Near spherical illumination of ion-beam and laser targets

    SciTech Connect

    Mark, J.W.K.

    1985-12-12

    A procedure is developed for reducing energy-deposition asymmetry in spherical targets driven directly by ion or laser beams. This work is part of a strategy for achieving illumination symmetry in such targets, which is proposed as an alternative to those in the literature. This strategy allows an axially symmetric placement of beamlets, which would be convenient for some driven or reactor scenarios. It also allows the use of beam currents or energy fluxes and beam transverse profiles to help reduce deposition asymmetry with fewer beamlets. In the ideal limit of thin deposition layers and controlled beam profiles, at most six beamlets are needed for target symmetry.

  16. Ion-assisted deposition processes for precision and laser optics

    NASA Astrophysics Data System (ADS)

    Ehlers, Henrik; Gross, Tobias; Lappschies, Marc; Ristau, Detlev

    2004-02-01

    As a consequence of the ever increasing application field of modern optical technologies, new demands for the optimization of deposition processes for high quality optical coatings with increased environmental stability and power handling capability are imposed on thin film manufacturers. Starting from this challenge, the presented work is focused on the development of an ion assisted deposition (IAD) process using a cold cathode ion source. Especially in the mid infrared wavelength region (MIR) with its water absorption bands, the ion assisted deposition process leads to many practical advantages, e.g. for medical laser applications. In the present study, a cold cathode ion source was operated with pure oxygen for the deposition of different oxide materials. Besides the determination of the optical properties, the characterization of the thin films included the first application of an in situ optical broadband monitoring system during the IAD process. The produced single layers and MIR coatings are thermally stable, shift-free, and exhibit lower absorption compared to conventionally deposited coatings. In contrast to the conventional coatings, also no vacuum-to-air shift is observed for the realized MIR coatings. Therefore, the stable and reproducible IAD process in combination with the new process control strategies using the broadband transmittance measurements on the moving substrates allows an advanced process control and a precise determination of the layer thickness.

  17. Measurement of beam characteristics from C{sup 6+} laser ion source

    SciTech Connect

    Yamaguchi, A. Sako, K.; Sato, K.; Hayashizaki, N.; Hattori, T.

    2014-02-15

    We developed a C{sup 6+} laser ion source for a heavy-ion accelerator. A carbon target was irradiated with a Q-switched Nd:YAG laser (1064 nm wavelength, 1.4 J maximum laser energy, 10 ns pulse duration) to generate a high-density plasma. The laser ion source employed a rotating carbon target for continuous operation. Ion beams were extracted from the plasma through a drift space using a direct plasma injection scheme [B. Yu. Sharkov, A. V. Shumshurov, V. P. Dubenkow, O. B. Shamaev, and A. A. Golubev, Rev. Sci. Instrum. 63, 2841 (1992)] up to a maximum voltage of 40 kV. We measured the characteristics of the ion beams from the laser ion source and present the results of experiments here.

  18. Control of laser-accelerated ions: Recent advances and preliminary results from the new Trident 250-TW laser

    NASA Astrophysics Data System (ADS)

    Hegelich, B. Manuel; Albright, Brian J.; Yin, Lin; Flippo, Kirk A.; Cort Gautier, D.; Letzring, Samuel; Schulze, Roland; Schmitt, Mark; Fernandez, Juan C.

    2007-11-01

    Advanced target design, treatment and characterization enable progress in laser-driven ion acceleration. We demonstrate spectral shaping and mono-energetic features from in-situ formed source layers on different substrate materials. Advanced targets and experimental techniques allow control of the properties of laser accelerated ion beams, which is of importance to future applications like Ion Fast Ignition (IFI), WDM research and others. We will also present preliminary results from the new 250-TW Trident laser system that will allow the extrapolation of scaling laws similar to those derived for proton acceleration.

  19. Laser desorption studies of high mass biomolecules in Fourier-transform ion cyclotron resonance mass spectrometry.

    PubMed Central

    Solouki, T; Russell, D H

    1992-01-01

    Matrix-assisted laser desorption ionization is used to obtain Fourier-transform ion cyclotron resonance mass spectra of model peptides (e.g., gramicidin S, angiotensin I, renin substrate, melittin, and bovine insulin). Matrix-assisted laser desorption ionization yields ions having appreciable kinetic energies. Two methods for trapping the high kinetic energy ions are described: (i) the ion signal for [M+H]+ ions is shown to increase with increasing trapping voltages, and (ii) collisional relaxation is used for the detection of [M+H]+ ions of bovine insulin. Images PMID:1378614

  20. Influence of laser pulse duration on extreme ultraviolet and ion emission features from tin plasmas

    SciTech Connect

    Roy, A. E-mail: aroy@barc.gov.in; Harilal, S. S.; Polek, M. P.; Hassan, S. M.; Hassanein, A.; Endo, A.

    2014-03-15

    We investigated the role of laser pulse duration and intensity on extreme ultraviolet (EUV) generation and ion emission from a laser produced Sn plasma. For producing plasmas, planar slabs of pure Sn were irradiated with 1064 nm Nd:YAG laser pulses with varying pulse duration (5–20 ns) and intensity. Experimental results performed at CMUXE indicate that the conversion efficiency (CE) of the EUV radiation strongly depend on laser pulse width and intensity, with a maximum CE of ∼2.0% measured for the shortest laser pulse width used (5 ns). Faraday Cup ion analysis of Sn plasma showed that the ion flux kinetic profiles are shifted to higher energy side with the reduction in laser pulse duration and narrower ion kinetic profiles are obtained for the longest pulse width used. However, our initial results showed that at a constant laser energy, the ion flux is more or less constant regardless of the excitation laser pulse width. The enhanced EUV emission obtained at shortest laser pulse duration studied is related to efficient laser-plasma reheating supported by presence of higher energy ions at these pulse durations.

  1. Emittance Characterization of a Hot-Cavity Laser Ion Source at HRIBF

    SciTech Connect

    Liu, Yuan; Baktash, Cyrus; Beene, James R; Havener, Charles C; Krause, Herbert F; Schultz, David Robert; Stracener, Daniel W; Vane, C Randy; Geppert, C.; Gottwald, T.; Kessler, T.; Wies, K.; Wendt, K.

    2009-01-01

    The first investigation of the transverse emittance of a hot-cavity laser ion source based on all-solid-state Ti:Sapphire lasers is presented. The emittances of 63Cu ion beams generated by three-photon resonant ionization are measured and compared with that of the 69Ga and 39K ion beams resulting from surface ionization in the same ion source. A Self-Consistent, Unbiased Elliptical Exclusion (SCUBEEx) method is adapted for noise reduction and emittance analysis. Typical values of the rms and 90% fractional emittances of the Cu ion beams at 20 keV energy are found to be about 2 -mm-mrad and 8 -mm-mrad, respectively, for the ion currents of 2 to 40 nA investigated. The emittances of the laser-produced Cu ion beams are smaller than those of the surface-ionized Ga and K ion beams.

  2. Self-proton/ion radiography of laser-produced proton/ion beam from thin foil targets

    SciTech Connect

    Paudel, Y.; Renard-Le Galloudec, N.; Kantsyrev, V. L.; Safronova, A. S.; Shrestha, I.; Osborne, G. C.; Shlyaptseva, V. V.; Sentoku, Y.; Nicolai, Ph.; D'Humieres, E.; Faenov, A.Ya.

    2012-12-15

    Protons and multicharged ions generated from high-intensity laser interactions with thin foil targets have been studied with a 100 TW laser system. Protons/ions with energies up to 10 MeV are accelerated either from the front or the rear surface of the target material. We have observed for the first time that the protons/ions accelerated from the front surface of the target, in a direction opposite to the laser propagation direction, are turned around and pulled back to the rear surface, in the laser propagation direction. This proton/ion beam is able to create a self-radiograph of the target and glass stalk holding the target itself recorded through the radiochromic film stack. This unique result indicates strong long-living (ns time scale) magnetic fields present in the laser-produced plasma, which are extremely important in energy transport during the intense laser irradiation. The magnetic field from laser main pulse expands rapidly in the preformed plasma to rotate the laser produced protons. Radiation hydrodynamic simulations and ray tracing found that the magnetic field created by the amplified spontaneous emission prepulse is not sufficient to explain the particle trajectories, but the additional field created by the main pulse interaction estimated from particle-in-cell simulation is able to change the particle trajectories.

  3. New methods for high current fast ion beam production by laser-driven acceleration

    SciTech Connect

    Margarone, D.; Krasa, J.; Prokupek, J.; Velyhan, A.; Laska, L.; Jungwirth, K.; Mocek, T.; Korn, G.; Rus, B.; Torrisi, L.; Gammino, S.; Cirrone, P.; Cutroneo, M.; Romano, F.; Picciotto, A.; Serra, E.; Giuffrida, L.; Mangione, A.; Rosinski, M.; Parys, P.; and others

    2012-02-15

    An overview of the last experimental campaigns on laser-driven ion acceleration performed at the PALS facility in Prague is given. Both the 2 TW, sub-nanosecond iodine laser system and the 20 TW, femtosecond Ti:sapphire laser, recently installed at PALS, are used along our experiments performed in the intensity range 10{sup 16}-10{sup 19} W/cm{sup 2}. The main goal of our studies was to generate high energy, high current ion streams at relatively low laser intensities. The discussed experimental investigations show promising results in terms of maximum ion energy and current density, which make the laser-accelerated ion beams a candidate for new-generation ion sources to be employed in medicine, nuclear physics, matter physics, and industry.

  4. Dynamics of ponderomotive ion acceleration in a laser-plasma channel

    SciTech Connect

    Kovalev, V. F.; Bychenkov, V. Yu.

    2015-04-15

    Analytical solution to the Cauchy problem for the kinetic equation describing the radial acceleration of ions under the action of the ponderomotive force of a laser beam undergoing guided propagation in transparent plasma is constructed. Spatial and temporal dependences of the ion distribution function and the integral ion characteristics, such as the density, average velocity, and energy spectrum, are obtained for an axisymmetric laser-plasma channel. The formation of a density peak near the channel boundary and the effect of ion flow breaking for a quasi-stationary laser beam are described analytically.

  5. Effect of active-ion concentration on holmium fibre laser efficiency

    SciTech Connect

    Kurkov, Andrei S; Sholokhov, E M; Marakulin, A V; Minashina, L A

    2010-08-03

    We have measured the fraction of holmium ions that relax nonradiatively to the ground level as a result of interaction at a metastable level in optical fibres with a silica-based core doped with holmium ions to 2 x 10{sup 19} - 2 x 10{sup 20} cm{sup -3}. The percentage of such ions has been shown to depend on the absolute active-ion concentration. The fibres have been used to make a number of 2.05-{mu}m lasers, and their slope efficiency has been measured. The laser efficiency decreases with increasing holmium concentration in the fibres (lasers)

  6. Proton beam production by a laser ion source with hydride target.

    PubMed

    Okamura, M; Stifler, C; Palm, K; Steski, D; Ikeda, S; Kumaki, M; Kanesue, T

    2016-02-01

    We studied proton beam production from a laser ion source using hydrogen rich target materials. In general, gas based species are not suitable for laser ion sources since formation of a dense laser target is difficult. In order to achieve reliable operation, we tested hydride targets using a sub nanosecond Q-switched Nd-YAG laser, which may help suppress target material consumption. We detected enough yields of protons from a titanium hydride target without degradation of beam current during the experiment. The combination of a sub nanosecond laser and compressed hydride target may provide stable proton beam. PMID:26931967

  7. First collinear laser spectroscopy measurements of radioisotopes from an IGISOL ion source

    NASA Astrophysics Data System (ADS)

    Billowes, J.; Campbell, P.; Cochrane, E. C. A.; Cooke, J. L.; Dendooven, P.; Evans, D. E.; Grant, I. S.; Griffith, J. A. R.; Honkanen, A.; Huhta, M.; Levins, J. M. G.; Liukkonen, E.; Oinonen, M.; Pearson, M. R.; Penttilä, H.; Persson, J. R.; Richardson, D. S.; Tungate, G.; Wheeler, P.; Zybert, L.; Äystö, J.

    The standard Doppler-free technique of collinear laser spectroscopy has been successfully applied to radioisotopes from the ion-guide isotope separator (IGISOL) at the University of Jyväskylä. The laser resonance fluorescence signals for the 140,142,144Ba radioisotopes show that the ion beam energy spread is less than 6 eV, allowing the laser technique to have both high resolution and a sensitivity comparable with the best obtained at conventional facilities.

  8. First collinear laser spectroscopy measurements of radioisotopes from an IGISOL ion source

    NASA Astrophysics Data System (ADS)

    Dendooven, P.; Honkenen, A.; Huhta, M.; Liukkonen, E.; Oinonen, M.; Penttilä, H.; Cochrane, E. C. A.; Cooke, J. L.; Evans, D. E.; Griffith, J. A. R.; Persson, J. R.; Richardson, D. S.; Tungate, G.; Zybert, L.; Billowes, J.; Campbell, P.; Grant, L. S.; Levins, J. M. G.; Pearson, M. R.; Wheeler, P.

    1996-04-01

    The standard Doppler-free technique of collinear laser spectroscopy has been successfully applied to radioisotopes from the ion-guide isotope separator (IGISOL) at the University of Jyväskylä. The laser resonance fluorescence signals for the a140,142,144Ba radioisotopes show that the ion beam energy spread is less than 6 eV, allowing the laser technique to have both high resolution and a sensitivity comparable with the best obtained at conventional facilities.

  9. Coulomb-driven energy boost of heavy ions for laser-plasma acceleration.

    PubMed

    Braenzel, J; Andreev, A A; Platonov, K; Klingsporn, M; Ehrentraut, L; Sandner, W; Schnürer, M

    2015-03-27

    An unprecedented increase of kinetic energy of laser accelerated heavy ions is demonstrated. Ultrathin gold foils have been irradiated by an ultrashort laser pulse at a peak intensity of 8×10^{19}  W/  cm^{2}. Highly charged gold ions with kinetic energies up to >200  MeV and a bandwidth limited energy distribution have been reached by using 1.3 J laser energy on target. 1D and 2D particle in cell simulations show how a spatial dependence on the ion's ionization leads to an enhancement of the accelerating electrical field. Our theoretical model considers a spatial distribution of the ionization inside the thin target, leading to a field enhancement for the heavy ions by Coulomb explosion. It is capable of explaining the energy boost of highly charged ions, enabling a higher efficiency for the laser-driven heavy ion acceleration.

  10. Coulomb-driven energy boost of heavy ions for laser-plasma acceleration.

    PubMed

    Braenzel, J; Andreev, A A; Platonov, K; Klingsporn, M; Ehrentraut, L; Sandner, W; Schnürer, M

    2015-03-27

    An unprecedented increase of kinetic energy of laser accelerated heavy ions is demonstrated. Ultrathin gold foils have been irradiated by an ultrashort laser pulse at a peak intensity of 8×10^{19}  W/  cm^{2}. Highly charged gold ions with kinetic energies up to >200  MeV and a bandwidth limited energy distribution have been reached by using 1.3 J laser energy on target. 1D and 2D particle in cell simulations show how a spatial dependence on the ion's ionization leads to an enhancement of the accelerating electrical field. Our theoretical model considers a spatial distribution of the ionization inside the thin target, leading to a field enhancement for the heavy ions by Coulomb explosion. It is capable of explaining the energy boost of highly charged ions, enabling a higher efficiency for the laser-driven heavy ion acceleration. PMID:25860747

  11. Direct heating of a laser-imploded core by ultraintense laser-driven ions.

    PubMed

    Kitagawa, Y; Mori, Y; Komeda, O; Ishii, K; Hanayama, R; Fujita, K; Okihara, S; Sekine, T; Satoh, N; Kurita, T; Takagi, M; Watari, T; Kawashima, T; Kan, H; Nishimura, Y; Sunahara, A; Sentoku, Y; Nakamura, N; Kondo, T; Fujine, M; Azuma, H; Motohiro, T; Hioki, T; Kakeno, M; Miura, E; Arikawa, Y; Nagai, T; Abe, Y; Ozaki, S; Noda, A

    2015-05-15

    A novel direct core heating fusion process is introduced, in which a preimploded core is predominantly heated by energetic ions driven by LFEX, an extremely energetic ultrashort pulse laser. Consequently, we have observed the D(d,n)^{3}He-reacted neutrons (DD beam-fusion neutrons) with the yield of 5×10^{8} n/4π sr. Examination of the beam-fusion neutrons verified that the ions directly collide with the core plasma. While the hot electrons heat the whole core volume, the energetic ions deposit their energies locally in the core, forming hot spots for fuel ignition. As evidenced in the spectrum, the process simultaneously excited thermal neutrons with the yield of 6×10^{7} n/4π sr, raising the local core temperature from 0.8 to 1.8 keV. A one-dimensional hydrocode STAR 1D explains the shell implosion dynamics including the beam fusion and thermal fusion initiated by fast deuterons and carbon ions. A two-dimensional collisional particle-in-cell code predicts the core heating due to resistive processes driven by hot electrons, and also the generation of fast ions, which could be an additional heating source when they reach the core. Since the core density is limited to 2 g/cm^{3} in the current experiment, neither hot electrons nor fast ions can efficiently deposit their energy and the neutron yield remains low. In future work, we will achieve the higher core density (>10 g/cm^{3}); then hot electrons could contribute more to the core heating via drag heating. Together with hot electrons, the ion contribution to fast ignition is indispensable for realizing high-gain fusion. By virtue of its core heating and ignition, the proposed scheme can potentially achieve high gain fusion. PMID:26024175

  12. Direct heating of a laser-imploded core by ultraintense laser-driven ions.

    PubMed

    Kitagawa, Y; Mori, Y; Komeda, O; Ishii, K; Hanayama, R; Fujita, K; Okihara, S; Sekine, T; Satoh, N; Kurita, T; Takagi, M; Watari, T; Kawashima, T; Kan, H; Nishimura, Y; Sunahara, A; Sentoku, Y; Nakamura, N; Kondo, T; Fujine, M; Azuma, H; Motohiro, T; Hioki, T; Kakeno, M; Miura, E; Arikawa, Y; Nagai, T; Abe, Y; Ozaki, S; Noda, A

    2015-05-15

    A novel direct core heating fusion process is introduced, in which a preimploded core is predominantly heated by energetic ions driven by LFEX, an extremely energetic ultrashort pulse laser. Consequently, we have observed the D(d,n)^{3}He-reacted neutrons (DD beam-fusion neutrons) with the yield of 5×10^{8} n/4π sr. Examination of the beam-fusion neutrons verified that the ions directly collide with the core plasma. While the hot electrons heat the whole core volume, the energetic ions deposit their energies locally in the core, forming hot spots for fuel ignition. As evidenced in the spectrum, the process simultaneously excited thermal neutrons with the yield of 6×10^{7} n/4π sr, raising the local core temperature from 0.8 to 1.8 keV. A one-dimensional hydrocode STAR 1D explains the shell implosion dynamics including the beam fusion and thermal fusion initiated by fast deuterons and carbon ions. A two-dimensional collisional particle-in-cell code predicts the core heating due to resistive processes driven by hot electrons, and also the generation of fast ions, which could be an additional heating source when they reach the core. Since the core density is limited to 2 g/cm^{3} in the current experiment, neither hot electrons nor fast ions can efficiently deposit their energy and the neutron yield remains low. In future work, we will achieve the higher core density (>10 g/cm^{3}); then hot electrons could contribute more to the core heating via drag heating. Together with hot electrons, the ion contribution to fast ignition is indispensable for realizing high-gain fusion. By virtue of its core heating and ignition, the proposed scheme can potentially achieve high gain fusion.

  13. Ambient pressure laser desorption and laser-induced acoustic desorption ion mobility spectrometry detection of explosives.

    PubMed

    Ehlert, Sven; Walte, Andreas; Zimmermann, Ralf

    2013-11-19

    The development of fast, mobile, and sensitive detection systems for security-relevant substances is of enormous importance. Because of the low vapor pressures of explosives and improvised explosive devices, adequate sampling procedures are crucial. Ion mobility spectrometers (IMSs) are fast and sensitive instruments that are used as detection systems for explosives. Ambient pressure laser desorption (APLD) and ambient pressure laser-induced acoustic desorption (AP-LIAD) are new tools suitable to evaporate explosives in order to detect them in the vapor phase. Indeed, the most important advantage of APLD or AP-LIAD is the capability to sample directly from the surface of interest without any transfer of the analyte to other surfaces such as wipe pads. A much more gentle desorption, compared to classical thermal-based desorption, is possible with laser-based desorption using very short laser pulses. With this approach the analyte molecules are evaporated in a very fast process, comparable to a shock wave. The thermal intake is reduced considerably. The functionality of APLD and AP-LIAD techniques combined with a hand-held IMS system is shown for a wide range of common explosives such as EGDN (ethylene glycol dinitrate), urea nitrate, PETN (pentaerythritol tetranitrate), HMTD (hexamethylene triperoxide diamine), RDX (hexogen), tetryl (2,4,6-trinitrophenylmethylnitramine), and TNT (trinitrotoluene). Detection limits down to the low nanogram range are obtained. The successful combination of IMS detection and APLD/AP-LIAD sampling is shown.

  14. Electron detachment from negative ions in a short laser pulse

    NASA Astrophysics Data System (ADS)

    Shearer, S. F. C.; Smyth, M. C.; Gribakin, G. F.

    2011-09-01

    We present an efficient and accurate method to study electron detachment from negative ions by a few-cycle linearly polarized laser pulse. The adiabatic saddle-point method of Gribakin and Kuchiev [Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.55.3760 55, 3760 (1997)] is adapted to calculate the transition amplitude for a short laser pulse. Its application to a pulse with N optical cycles produces 2(N+1) saddle points in complex time, which form a characteristic “smile.” Numerical calculations are performed for H- in a 5-cycle pulse with frequency 0.0043 a.u. and intensities of 1010, 5×1010, and 1011 W/cm2, and for various carrier-envelope phases. We determine the spectrum of the photoelectrons as a function of both energy and emission angle, as well as the angle-integrated energy spectra and total detachment probabilities. Our calculations show that the dominant contribution to the transition amplitude is given by 5-6 central saddle points, which correspond to the strongest part of the pulse. We examine the dependence of the photoelectron angular distributions on the carrier-envelope phase and show that measuring such distributions can provide a way of determining this phase.

  15. Electron detachment from negative ions in a short laser pulse

    SciTech Connect

    Shearer, S. F. C.; Smyth, M. C.; Gribakin, G. F.

    2011-09-15

    We present an efficient and accurate method to study electron detachment from negative ions by a few-cycle linearly polarized laser pulse. The adiabatic saddle-point method of Gribakin and Kuchiev [Phys. Rev. A 55, 3760 (1997)] is adapted to calculate the transition amplitude for a short laser pulse. Its application to a pulse with N optical cycles produces 2(N+1) saddle points in complex time, which form a characteristic 'smile.' Numerical calculations are performed for H{sup -} in a 5-cycle pulse with frequency 0.0043 a.u. and intensities of 10{sup 10}, 5x10{sup 10}, and 10{sup 11} W/cm{sup 2}, and for various carrier-envelope phases. We determine the spectrum of the photoelectrons as a function of both energy and emission angle, as well as the angle-integrated energy spectra and total detachment probabilities. Our calculations show that the dominant contribution to the transition amplitude is given by 5-6 central saddle points, which correspond to the strongest part of the pulse. We examine the dependence of the photoelectron angular distributions on the carrier-envelope phase and show that measuring such distributions can provide a way of determining this phase.

  16. Ion implanted and laser processed solar cells made from EFG ribbon

    SciTech Connect

    Ladd, L. A.; Ravi, K. V.; Narayan, J.

    1980-01-01

    The use of ion implantation and laser processing has a number of conceptual advantages which could result in a low-cost process for manufacturing high performance solar cells from EFG ribbon. Samples were phosphorus ion implanted, laser processed using either a pulse large area ruby laser or a scanned YAG laser with a second harmonic generator, and then processed into solar cells. Many of the samples had high reverse leakage and it was determined that this was due to too high a laser processing power. This effect was determined to be more severe for the scanned YAG laser, and is thought to be due to point defects. Cells were made from EFG ribbon with a low laser energy density which had efficiencies of up to 10% at AMI demonstrating the feasibility of this approach. High efficiencies should be attainable by optimizing the laser processing parameters.

  17. On-line surfactant monitoring

    SciTech Connect

    Mullen, K.I.; Neal, E.E.; Soran, P.D.; Smith, B.

    1995-04-01

    This group has developed a process to extract metal ions from dilute aqueous solutions. The process uses water soluble polymers to complex metal ions. The metal/polymer complex is concentrated by ultrafiltration and the metals are recovered by a pH adjustment that frees the metal ions. The metal ions pass through the ultrafiltration membrane and are recovered in a concentrated form suitable for reuse. Surfactants are present in one of the target waste streams. Surfactants foul the costly ultrafiltration membranes. It was necessary to remove the surfactants before processing the waste stream. This paper discusses an on-line device the authors fabricated to monitor the process stream to assure that all the surfactant had been removed. The device is inexpensive and sensitive to very low levels of surfactants.

  18. Ionization, ion distribution, and ion focusing in laser plasmas from atomic and diatomic targets

    SciTech Connect

    Srivastava, S. N.; Rohr, K.; Sinha, B. K.

    2006-04-01

    Charge-resolved measurements of the total number of particles from plasmas produced from planar, monoatomic targets of copper and tungsten as well as the binary targets of copper and tungsten are reported, using a 125 mJ, 5 ns, Nd:YAG laser, at a laser intensity of about 10{sup 10} W/cm{sup 2}. The measurements show a severe quenching of the ionization states in the case of the diatomic targets. These measurements and their variations with ionization state support the theoretical investigations of plasma motion under the influence of the viscous force in case of plasmas consisting of light and heavy particles. Gaussian width measurements of the angular particle distribution showed a focusing effect towards the target normal, the width decreasing as the ion mass and ionization state increased. From the analysis of the theoretical results on self-similarity expansion it is concluded that the ion acceleration due to the built-in electrostatic potential is not significant.

  19. Beamed neutron emission driven by laser accelerated light ions

    NASA Astrophysics Data System (ADS)

    Kar, S.; Green, A.; Ahmed, H.; Alejo, A.; Robinson, A. P. L.; Cerchez, M.; Clarke, R.; Doria, D.; Dorkings, S.; Fernandez, J.; Mirfayzi, S. R.; McKenna, P.; Naughton, K.; Neely, D.; Norreys, P.; Peth, C.; Powell, H.; Ruiz, J. A.; Swain, J.; Willi, O.; Borghesi, M.

    2016-05-01

    Highly anisotropic, beam-like neutron emission with peak flux of the order of 109 n/sr was obtained from light nuclei reactions in a pitcher-catcher scenario, by employing MeV ions driven by a sub-petawatt laser. The spatial profile of the neutron beam, fully captured for the first time by employing a CR39 nuclear track detector, shows a FWHM divergence angle of ˜ 70^\\circ , with a peak flux nearly an order of magnitude higher than the isotropic component elsewhere. The observed beamed flux of neutrons is highly favourable for a wide range of applications, and indeed for further transport and moderation to thermal energies. A systematic study employing various combinations of pitcher-catcher materials indicates the dominant reactions being d(p, n+p)1H and d(d,n)3He. Albeit insufficient cross-section data are available for modelling, the observed anisotropy in the neutrons’ spatial and spectral profiles is most likely related to the directionality and high energy of the projectile ions.

  20. Rapid Screening of Carboxylic Acids from Waste and Surface Waters by ESI-MS/MS Using Barium Ion Chemistry and On-Line Membrane Sampling.

    PubMed

    Duncan, Kyle D; Volmer, Dietrich A; Gill, Chris G; Krogh, Erik T

    2016-03-01

    Negative ion tandem mass spectrometric analysis of aliphatic carboxylic acids often yields only non-diagnostic ([M - H](-)) ions with limited selective fragmentation. However, carboxylates cationized with Ba(2+) have demonstrated efficient dissociation in positive ion mode, providing structurally diagnostic product ions. We report the application of barium adducts followed by collision induced dissociation (CID), to improve selectivity for rapid screening of carboxylic acids in complex aqueous samples. The quantitative MS/MS method presented utilizes common product ions of [M - H + Ba](+) precursor ions. The mechanism of product ion formation is investigated using isotopically labeled standards and a series of structurally related carboxylic acids. The results suggest that hydrogen atoms in the β and γ positions yield common product ions ([BaH](+) and [BaOH](+)). Furthermore, the diagnostic product ion at m/z 196 serves as a qualifying ion for carboxylate species. This methodology has been successfully used in conjunction with condensed phase membrane introduction mass spectrometry (CP-MIMS), with barium acetate added directly to the methanol acceptor phase. The combination enables rapid screening of carboxylic acids directly from acidified water samples (wastewater effluent, spiked natural waters) using a capillary hollow fiber PDMS membrane immersion probe. We have applied this technique for the direct analysis of complex naphthenic acid mixtures spiked into natural surface waters using CP-MIMS. Selectivity at the ionization and tandem mass spectrometry level eliminate isobaric interferences from hydroxylated species present within the samples, which have been observed in negative electrospray ionization.

  1. Rapid Screening of Carboxylic Acids from Waste and Surface Waters by ESI-MS/MS Using Barium Ion Chemistry and On-Line Membrane Sampling

    NASA Astrophysics Data System (ADS)

    Duncan, Kyle D.; Volmer, Dietrich A.; Gill, Chris G.; Krogh, Erik T.

    2016-03-01

    Negative ion tandem mass spectrometric analysis of aliphatic carboxylic acids often yields only non-diagnostic ([M - H]-) ions with limited selective fragmentation. However, carboxylates cationized with Ba2+ have demonstrated efficient dissociation in positive ion mode, providing structurally diagnostic product ions. We report the application of barium adducts followed by collision induced dissociation (CID), to improve selectivity for rapid screening of carboxylic acids in complex aqueous samples. The quantitative MS/MS method presented utilizes common product ions of [M - H + Ba]+ precursor ions. The mechanism of product ion formation is investigated using isotopically labeled standards and a series of structurally related carboxylic acids. The results suggest that hydrogen atoms in the β and γ positions yield common product ions ([BaH]+ and [BaOH]+). Furthermore, the diagnostic product ion at m/z 196 serves as a qualifying ion for carboxylate species. This methodology has been successfully used in conjunction with condensed phase membrane introduction mass spectrometry (CP-MIMS), with barium acetate added directly to the methanol acceptor phase. The combination enables rapid screening of carboxylic acids directly from acidified water samples (wastewater effluent, spiked natural waters) using a capillary hollow fiber PDMS membrane immersion probe. We have applied this technique for the direct analysis of complex naphthenic acid mixtures spiked into natural surface waters using CP-MIMS. Selectivity at the ionization and tandem mass spectrometry level eliminate isobaric interferences from hydroxylated species present within the samples, which have been observed in negative electrospray ionization.

  2. Instrumentation for diagnostics and control of laser-accelerated proton (ion) beams.

    PubMed

    Bolton, P R; Borghesi, M; Brenner, C; Carroll, D C; De Martinis, C; Fiorini, Francesca; Flacco, A; Floquet, V; Fuchs, J; Gallegos, P; Giove, D; Green, J S; Green, S; Jones, B; Kirby, D; McKenna, P; Neely, D; Nuesslin, F; Prasad, R; Reinhardt, S; Roth, M; Schramm, U; Scott, G G; Ter-Avetisyan, S; Tolley, M; Turchetti, G; Wilkens, J J

    2014-05-01

    Suitable instrumentation for laser-accelerated proton (ion) beams is critical for development of integrated, laser-driven ion accelerator systems. Instrumentation aimed at beam diagnostics and control must be applied to the driving laser pulse, the laser-plasma that forms at the target and the emergent proton (ion) bunch in a correlated way to develop these novel accelerators. This report is a brief overview of established diagnostic techniques and new developments based on material presented at the first workshop on 'Instrumentation for Diagnostics and Control of Laser-accelerated Proton (Ion) Beams' in Abingdon, UK. It includes radiochromic film (RCF), image plates (IP), micro-channel plates (MCP), Thomson spectrometers, prompt inline scintillators, time and space-resolved interferometry (TASRI) and nuclear activation schemes. Repetition-rated instrumentation requirements for target metrology are also addressed.

  3. Spatiotemporal dynamics of Gaussian laser pulse in a multi ions plasma

    NASA Astrophysics Data System (ADS)

    Jafari Milani, M. R.

    2016-08-01

    Spatiotemporal evolutions of Gaussian laser pulse propagating through a plasma with multiple charged ions are studied, taking into account the ponderomotive nonlinearity. Coupled differential equations for beam width and pulse length parameters are established and numerically solved using paraxial ray approximation. In one-dimensional geometry, effects of laser and plasma parameters such as laser intensity, plasma density, and temperature on the longitudinal pulse compression and the laser intensity distribution are analyzed for plasmas with singly and doubly charged ions. The results demonstrate that self-compression occurs in a laser intensity range with a turning point intensity in which the self-compression process has its strongest extent. The results also show that the multiply ionized ions have different effect on the pulse compression above and below turning point intensity. Finally, three-dimensional geometry is used to analyze the simultaneous evolution of both self-focusing and self-compression of Gaussian laser pulse in such plasmas.

  4. Efficient quasi-monoenergetic ion beams from laser-driven relativistic plasmas.

    PubMed

    Palaniyappan, Sasi; Huang, Chengkun; Gautier, Donald C; Hamilton, Christopher E; Santiago, Miguel A; Kreuzer, Christian; Sefkow, Adam B; Shah, Rahul C; Fernández, Juan C

    2015-01-01

    Table-top laser-plasma ion accelerators have many exciting applications, many of which require ion beams with simultaneous narrow energy spread and high conversion efficiency. However, achieving these requirements has been elusive. Here we report the experimental demonstration of laser-driven ion beams with narrow energy spread and energies up to 18 MeV per nucleon and ∼5% conversion efficiency (that is 4 J out of 80-J laser). Using computer simulations we identify a self-organizing scheme that reduces the ion energy spread after the laser exits the plasma through persisting self-generated plasma electric (∼10(12) V m(-1)) and magnetic (∼10(4) T) fields. These results contribute to the development of next generation compact accelerators suitable for many applications such as isochoric heating for ion-fast ignition and producing warm dense matter for basic science. PMID:26657147

  5. Ion acceleration by intense, few-cycle laser pulses with nanodroplets

    SciTech Connect

    Di Lucchio, Laura; Andreev, Alexander A.; Gibbon, Paul

    2015-05-15

    The energy distribution of electrons and ions emerging from the interaction of a few-cycle Gaussian laser pulse with spherical nanoclusters is investigated with the aim of determining prospects for accelerating ions in this regime. It is found that the direct conversion of laser energy into dense attosecond electron nanobunches results in rapid charge separation and early onset of Coulomb-explosion-dominated ion dynamics. The ion core of the cluster starts to expand soon after the laser has crossed the droplet, the fastest ions attaining 10 s of MeV at relativistic intensities. The current investigation should serve as a guide for contemporary experiments, i.e., using state-of-the-art few-cycle ultraintense lasers and nanoclusters of solid density.

  6. Effect of the active-ion concentration on the lasing dynamics of holmium fibre lasers

    SciTech Connect

    Kurkov, Andrei S; Sholokhov, E M; Marakulin, A V; Minashina, L A

    2010-12-09

    The lasing dynamics of fibre lasers with a core based on quartz glass doped with holmium ions to concentrations in the range of 10{sup 19}-10{sup 20} cm{sup -3} is investigated. It is shown that fibre lasers with a high concentration of active holmium ions generate pulses, but a decrease in the holmium concentration changes the lasing from pulsed to cw regime. At the same time, a decrease in the active-ion concentration and the corresponding increase in the fibre length in the cavity reduce the lasing efficiency. (lasers)

  7. Dependence of multiply charged ions on the polarization state in nanosecond laser-benzene cluster interaction

    NASA Astrophysics Data System (ADS)

    Wang, Weiguo; Zhao, Wuduo; Hua, Lei; Hou, Keyong; Li, Haiyang

    2016-05-01

    This paper investigated the dependence of multiply charged ions on the laser polarization state when benzene cluster was irradiated with 532 and 1064 nm nanosecond laser. A circle, square and flower distribution for C2+, C3+ and C4+ were observed with 532 nm laser respectively, while flower petals for C2+, C3+ and C4+ were observed at 1064 nm as the laser polarization varied. A theoretical calculation was performed to interpret the polarization state and wavelength dependence of the multiply charged ions. The simulated results agreed well with the experimental observation with considering the contribution from the cluster disintegration.

  8. A long-term frequency stabilized deep ultraviolet laser for Mg+ ions trapping experiments

    NASA Astrophysics Data System (ADS)

    Zhang, J.; Yuan, W. H.; Deng, K.; Deng, A.; Xu, Z. T.; Qin, C. B.; Lu, Z. H.; Luo, J.

    2013-12-01

    As many precision laser spectroscopy experiments require frequency stabilized lasers, development of long-term stabilized lasers is of great interest. In this work, we report long-term frequency stabilization of a 280 nm deep ultraviolet laser to a high precision wavemeter with digital servo control such that the long-term drift of the laser frequency was greatly reduced. Long-term laser frequency drift was measured with a fiber frequency comb system over 8 h. After locking, the maximum drift rate of the 280 nm laser was lowered from 576 MHz/h to 6.4 MHz/h. With proper environment control of the wavemeter, the maximum drift rate of the 280 nm laser was further lowered to less than 480 kHz/h. The locked laser system was successfully used in a Mg+ ions trapping experiment, which was also discussed in this work.

  9. A long-term frequency stabilized deep ultraviolet laser for Mg+ ions trapping experiments.

    PubMed

    Zhang, J; Yuan, W H; Deng, K; Deng, A; Xu, Z T; Qin, C B; Lu, Z H; Luo, J

    2013-12-01

    As many precision laser spectroscopy experiments require frequency stabilized lasers, development of long-term stabilized lasers is of great interest. In this work, we report long-term frequency stabilization of a 280 nm deep ultraviolet laser to a high precision wavemeter with digital servo control such that the long-term drift of the laser frequency was greatly reduced. Long-term laser frequency drift was measured with a fiber frequency comb system over 8 h. After locking, the maximum drift rate of the 280 nm laser was lowered from 576 MHz/h to 6.4 MHz/h. With proper environment control of the wavemeter, the maximum drift rate of the 280 nm laser was further lowered to less than 480 kHz/h. The locked laser system was successfully used in a Mg(+) ions trapping experiment, which was also discussed in this work.

  10. Formation of Metal-Related Ions in Matrix-Assisted Laser Desorption Ionization.

    PubMed

    Lee, Chuping; Lu, I-Chung; Hsu, Hsu Chen; Lin, Hou-Yu; Liang, Sheng-Ping; Lee, Yuan-Tseh; Ni, Chi-Kung

    2016-09-01

    In a study of the metal-related ion generation mechanism in matrix-assisted laser desorption ionization (MALDI), crystals of matrix used in MALDI were grown from matrix- and salt-containing solutions. The intensities of metal ion and metal adducts of the matrix ion obtained from unwashed crystals were higher than those from crystals washed with deionized water, indicating that metal ions and metal adducts of the matrix ions are mainly generated from the surface of crystals. The contributions of preformed metal ions and metal adducts of the matrix ions inside the matrix crystals were minor. Metal adducts of the matrix and analyte ion intensities generated from a mixture of dried matrix, salt, and analyte powders were similar to or higher than those generated from the powder of dried droplet crystals, indicating that the contributions of the preformed metal adducts of the matrix and analyte ions were insignificant. Correlation between metal-related ion intensity fluctuation and protonated ion intensity fluctuation was observed, indicating that the generation mechanism of the metal-related ions is similar to that of the protonated ions. Because the thermally induced proton transfer model effectively describes the generation of the protonated ions, we suggest that metal-related ions are mainly generated from the salt dissolution in the matrix melted by the laser. Graphical Abstract ᅟ.

  11. Formation of Metal-Related Ions in Matrix-Assisted Laser Desorption Ionization

    NASA Astrophysics Data System (ADS)

    Lee, Chuping; Lu, I.-Chung; Hsu, Hsu Chen; Lin, Hou-Yu; Liang, Sheng-Ping; Lee, Yuan-Tseh; Ni, Chi-Kung

    2016-09-01

    In a study of the metal-related ion generation mechanism in matrix-assisted laser desorption ionization (MALDI), crystals of matrix used in MALDI were grown from matrix- and salt-containing solutions. The intensities of metal ion and metal adducts of the matrix ion obtained from unwashed crystals were higher than those from crystals washed with deionized water, indicating that metal ions and metal adducts of the matrix ions are mainly generated from the surface of crystals. The contributions of preformed metal ions and metal adducts of the matrix ions inside the matrix crystals were minor. Metal adducts of the matrix and analyte ion intensities generated from a mixture of dried matrix, salt, and analyte powders were similar to or higher than those generated from the powder of dried droplet crystals, indicating that the contributions of the preformed metal adducts of the matrix and analyte ions were insignificant. Correlation between metal-related ion intensity fluctuation and protonated ion intensity fluctuation was observed, indicating that the generation mechanism of the metal-related ions is similar to that of the protonated ions. Because the thermally induced proton transfer model effectively describes the generation of the protonated ions, we suggest that metal-related ions are mainly generated from the salt dissolution in the matrix melted by the laser.

  12. Multidiagnostics analysis of ion dynamics in ultrafast laser ablation of metals over a large fluence range

    SciTech Connect

    Anoop, K. K.; Polek, M. P.; Bruzzese, R.; Amoruso, S.; Harilal, Sivanandan S.

    2015-02-28

    The ions dynamics in ultrafast laser ablation of metals is studied over a fluence range spanning from the ablation threshold up to ~75 J/cm2 by means of three established diagnostic techniques. Langmuir probe, Faraday cup and spectrally resolved ICCD imaging simultaneously monitor the laser-produced plasma ions produced during ultrafast laser ablation of a copper target. The fluence dependence of ion yield is analyzed observing the occurrence of three different regimes. Moreover, the specific ion yield shows a maximum at about 4-5 J/cm2, followed by a gradual reduction and a transition to a high-fluence regime above ~50 J/cm2. The fluence variation of the copper ions angular distribution is also analyzed, observing a gradual increase of forward peaking of Cu ions for fluences up to ~10 J/cm2. Then, a broader ion component is observed at larger angles for fluences larger than ~10 J/cm2. Finally, an experimental characterization of the ions angular distribution for several metallic targets (Mg, Al, Cr, Fe, Cu, and W) is carried out at a relatively high fluence of ~66 J/cm2. Interestingly, the ion emission from the volatile metals show a narrow forward peaked distribution and a high peak ion yield compared to the refractory metals. Moreover, the width of ion angular distributions presents a striking correlation with the peak ion yield.

  13. Intense laser driven collision-less shock and ion acceleration in magnetized plasmas

    NASA Astrophysics Data System (ADS)

    Mima, K.; Jia, Q.; Cai, H. B.; Taguchi, T.; Nagatomo, H.; Sanz, J. R.; Honrubia, J.

    2016-05-01

    The generation of strong magnetic field with a laser driven coil has been demonstrated by many experiments. It is applicable to the magnetized fast ignition (MFI), the collision-less shock in the astrophysics and the ion shock acceleration. In this paper, the longitudinal magnetic field effect on the shock wave driven by the radiation pressure of an intense short pulse laser is investigated by theory and simulations. The transition of a laminar shock (electro static shock) to the turbulent shock (electromagnetic shock) occurs, when the external magnetic field is applied in near relativistic cut-off density plasmas. This transition leads to the enhancement of conversion of the laser energy into high energy ions. The enhancement of the conversion efficiency is important for the ion driven fast ignition and the laser driven neutron source. It is found that the total number of ions reflected by the shock increases by six time when the magnetic field is applied.

  14. Guided post-acceleration of laser-driven ions by a miniature modular structure

    NASA Astrophysics Data System (ADS)

    Kar, Satyabrata; Ahmed, Hamad; Prasad, Rajendra; Cerchez, Mirela; Brauckmann, Stephanie; Aurand, Bastian; Cantono, Giada; Hadjisolomou, Prokopis; Lewis, Ciaran L. S.; Macchi, Andrea; Nersisyan, Gagik; Robinson, Alexander P. L.; Schroer, Anna M.; Swantusch, Marco; Zepf, Matt; Willi, Oswald; Borghesi, Marco

    2016-04-01

    All-optical approaches to particle acceleration are currently attracting a significant research effort internationally. Although characterized by exceptional transverse and longitudinal emittance, laser-driven ion beams currently have limitations in terms of peak ion energy, bandwidth of the energy spectrum and beam divergence. Here we introduce the concept of a versatile, miniature linear accelerating module, which, by employing laser-excited electromagnetic pulses directed along a helical path surrounding the laser-accelerated ion beams, addresses these shortcomings simultaneously. In a proof-of-principle experiment on a university-scale system, we demonstrate post-acceleration of laser-driven protons from a flat foil at a rate of 0.5 GeV m-1, already beyond what can be sustained by conventional accelerator technologies, with dynamic beam collimation and energy selection. These results open up new opportunities for the development of extremely compact and cost-effective ion accelerators for both established and innovative applications.

  15. Bicircular-laser-field-assisted electron-ion radiative recombination

    NASA Astrophysics Data System (ADS)

    Odžak, S.; Milošević, D. B.

    2015-11-01

    Electron-ion radiative recombination assisted by a bicircular laser field that consists of two circularly polarized fields counterrotating in the x y plane and having the frequencies r ω and s ω , which are integer multiples of the fundamental frequency ω , is considered using the S -matrix theory. The energy and polarization of soft x rays generated in this process are analyzed as functions of the incident electron energy and incident electron angle with respect to the x axis. Numerical results for the process of direct recombination of electrons with He+ ionic targets are presented. Abrupt cutoffs of the plateau structures in the emitted x-ray energy spectra are explained by classical analysis. Simpler or more complex oscillatory structures in the spectrum may appear as a result of the interference of a different number of classical orbits. Symmetry analysis and the numerical results show that the x-ray power spectrum and ellipticity are invariant with respect to a rotation of the incident electron momentum by the angle 2 π /(r +s ) . We have visualized this by presenting the logarithm of the differential power spectrum and polarization of the emitted x rays in false colors as functions of the incident electron angle and the x-ray energy. We have also shown that the change of the relative phase of the bicircular field is equivalent to the change of the incident electron angle. By controlling this relative phase it is possible to control the polarization of the emitted soft x rays.

  16. Laser ion source with long pulse width for RHIC-EBIS

    SciTech Connect

    Kondo, K.; Kanesue, T.; Okamura, M.

    2011-03-28

    The Electron Beam Ion Source (EBIS) at Brookhaven National Laboratory is a new heavy ion-projector for RHIC and NASA Space Radiation Laboratory. Laser Ion Source (LIS) with solenoid can supply many kinds of ion from solid targets and is suitable for long pulse length with low current as ion provider for RHIC-EBIS. In order to understand a plasma behavior for fringe field of solenoid, we measure current, pulse width and total ion charges by a new ion probe. The experimental result indicates that the solenoid confines the laser ablation plasma transversely. Laser ion source needs long pulse length with limited current as primary ion provider for RHIC-EBIS. New ion probe can measure current distribution for the radial positions along z axis. The beam pulse length is not effected by magnetic field strength. However, the currents and charges decay with the distance from the end of solenoid. These results indicate that solenoid field has important role for plasma confinement not longitudinally but transversely and solenoid is able to have long pulse length with sufficient total ion charges. Moreover, the results are useful for a design of the extraction system for RHIC-EBIS.

  17. Development of the C{sup 6+} laser ablation ion source for the KEK digital accelerator

    SciTech Connect

    Munemoto, Naoya; Takayama, Ken; Takano, Susumu; Okamura, Masahiro; Kumaki, Masahumi

    2014-02-15

    A laser ion source that provides a fully ionized carbon ion beam is under joint development at the High Energy Accelerator Research Organization and Brookhaven National Laboratory. Long-pulse (6 ns) and short-pulse (500 ps) laser systems were tested by using them to irradiate a graphite target. Notable differences between the systems were observed in these experiments. Preliminary experimental results, such as the charge-state spectrum, beam intensity, and stability, are discussed.

  18. Status of Real-Time Laser Based Ion Engine Diagnostics at NASA Glenn Research Center

    NASA Technical Reports Server (NTRS)

    Domonkos, Matthew T.; Williams, George J., Jr.

    2001-01-01

    The development status of laser based erosion diagnostics for ion engines at the NASA Glenn Research Center is discussed. The diagnostics are being developed to enhance component life-prediction capabilities. A direct measurement of the erosion product density using laser induced fluorescence (LIF) is described. Erosion diagnostics based upon evaluation of the ion dynamics are also under development, and the basic approach is presented. The planned implementation of the diagnostics is discussed.

  19. Invited Review Article: "Hands-on" laser-driven ion acceleration: A primer for laser-driven source development and potential applications.

    PubMed

    Schreiber, J; Bolton, P R; Parodi, K

    2016-07-01

    An overview of progress and typical yields from intense laser-plasma acceleration of ions is presented. The evolution of laser-driven ion acceleration at relativistic intensities ushers prospects for improved functionality and diverse applications which can represent a varied assortment of ion beam requirements. This mandates the development of the integrated laser-driven ion accelerator system, the multiple components of which are described. Relevant high field laser-plasma science and design of controlled optimum pulsed laser irradiation on target are dominant single shot (pulse) considerations with aspects that are appropriate to the emerging petawatt era. The pulse energy scaling of maximum ion energies and typical differential spectra obtained over the past two decades provide guidance for continued advancement of laser-driven energetic ion sources and their meaningful applications. PMID:27475539

  20. Invited Review Article: "Hands-on" laser-driven ion acceleration: A primer for laser-driven source development and potential applications

    NASA Astrophysics Data System (ADS)

    Schreiber, J.; Bolton, P. R.; Parodi, K.

    2016-07-01

    An overview of progress and typical yields from intense laser-plasma acceleration of ions is presented. The evolution of laser-driven ion acceleration at relativistic intensities ushers prospects for improved functionality and diverse applications which can represent a varied assortment of ion beam requirements. This mandates the development of the integrated laser-driven ion accelerator system, the multiple components of which are described. Relevant high field laser-plasma science and design of controlled optimum pulsed laser irradiation on target are dominant single shot (pulse) considerations with aspects that are appropriate to the emerging petawatt era. The pulse energy scaling of maximum ion energies and typical differential spectra obtained over the past two decades provide guidance for continued advancement of laser-driven energetic ion sources and their meaningful applications.

  1. Preferential enhancement of laser-driven carbon ion acceleration from optimized nanostructured surfaces

    PubMed Central

    Dalui, Malay; Wang, W.-M.; Trivikram, T. Madhu; Sarkar, Subhrangshu; Tata, Sheroy; Jha, J.; Ayyub, P.; Sheng, Z. M.; Krishnamurthy, M.

    2015-01-01

    High-intensity ultrashort laser pulses focused on metal targets readily generate hot dense plasmas which accelerate ions efficiently and can pave way to compact table-top accelerators. Laser-driven ion acceleration studies predominantly focus on protons, which experience the maximum acceleration owing to their highest charge-to-mass ratio. The possibility of tailoring such schemes for the preferential acceleration of a particular ion species is very much desired but has hardly been explored. Here, we present an experimental demonstration of how the nanostructuring of a copper target can be optimized for enhanced carbon ion acceleration over protons or Cu-ions. Specifically, a thin (≈0.25 μm) layer of 25–30 nm diameter Cu nanoparticles, sputter-deposited on a polished Cu-substrate, enhances the carbon ion energy by about 10-fold at a laser intensity of 1.2×1018  W/cm2. However, particles smaller than 20 nm have an adverse effect on the ion acceleration. Particle-in-cell simulations provide definite pointers regarding the size of nanoparticles necessary for maximizing the ion acceleration. The inherent contrast of the laser pulse is found to play an important role in the species selective ion acceleration. PMID:26153048

  2. Angular ion species distribution in droplet-based laser-produced plasmas

    SciTech Connect

    Giovannini, Andrea Z.; Gambino, Nadia; Rollinger, Bob; Abhari, Reza S.

    2015-01-21

    The angular distribution of the ion species generated from a laser irradiated droplet target is measured. The employed instrument was an electrostatic energy analyzer with differential pumping. Singly and doubly charged ions were detected at an argon ambient gas pressure of 2 × 10{sup −2} mbar. The amount of Sn{sup +} and Sn{sup 2+} and their kinetic energy is measured from 45° to 120° from the laser axis. Sn{sup +} expands approximately isotropically, and Sn{sup 2+} expansion is peaked towards the incoming laser radiation. The singly charged ion kinetic energy is close to constant over the measurement range, while it decreases by around 30% for Sn{sup 2+}. A calibrated model of the ion expansion that includes recombinations correctly predicts the mean ion charge distribution. The model is able to qualitatively estimate the influence of the laser wavelength on the mean ion charge distribution. The results show a more pronounced isotropic distribution for shorter wavelengths, and a more forward-peaked distribution for longer wavelengths. The ion charge distribution expected without the ambient gas is estimated through the measured ion kinetic energy. The presence of the ambient gas results in a decrease of the mean ion charge state and a decrease in angular anisotropy.

  3. Preferential enhancement of laser-driven carbon ion acceleration from optimized nanostructured surfaces.

    PubMed

    Dalui, Malay; Wang, W-M; Trivikram, T Madhu; Sarkar, Subhrangsu; Sarkar, Subhrangshu; Tata, Sheroy; Jha, J; Ayyub, P; Sheng, Z M; Krishnamurthy, M

    2015-01-01

    High-intensity ultrashort laser pulses focused on metal targets readily generate hot dense plasmas which accelerate ions efficiently and can pave way to compact table-top accelerators. Laser-driven ion acceleration studies predominantly focus on protons, which experience the maximum acceleration owing to their highest charge-to-mass ratio. The possibility of tailoring such schemes for the preferential acceleration of a particular ion species is very much desired but has hardly been explored. Here, we present an experimental demonstration of how the nanostructuring of a copper target can be optimized for enhanced carbon ion acceleration over protons or Cu-ions. Specifically, a thin (≈ 0.25 μm) layer of 25-30 nm diameter Cu nanoparticles, sputter-deposited on a polished Cu-substrate, enhances the carbon ion energy by about 10-fold at a laser intensity of 1.2 × 10(18)  W/cm(2). However, particles smaller than 20 nm have an adverse effect on the ion acceleration. Particle-in-cell simulations provide definite pointers regarding the size of nanoparticles necessary for maximizing the ion acceleration. The inherent contrast of the laser pulse is found to play an important role in the species selective ion acceleration. PMID:26153048

  4. Multiple species beam production on laser ion source for electron beam ion source in Brookhaven National Laboratory

    SciTech Connect

    Sekine, M.; Ikeda, S.; Hayashizaki, N.; Kanesue, T.; Okamura, M.

    2014-02-15

    Extracted ion beams from the test laser ion source (LIS) were transported through a test beam transport line which is almost identical to the actual primary beam transport in the current electron beam ion source apparatus. The tested species were C, Al, Si, Cr, Fe, Cu, Ag, Ta, and Au. The all measured beam currents fulfilled the requirements. However, in the case of light mass ions, the recorded emittance shapes have larger aberrations and the RMS values are higher than 0.06 π mm mrad, which is the design goal. Since we have margin to enhance the beam current, if we then allow some beam losses at the injection point, the number of the single charged ions within the acceptance can be supplied. For heaver ions like Ag, Ta, and Au, the LIS showed very good performance.

  5. Break-out afterburner ion acceleration in the longer laser pulse length regime

    SciTech Connect

    Yin, L.; Albright, B. J.; Shah, R. C.; Palaniyappan, S.; Fernndez, J. C.; Jung, D.; Henig, A.; Bowers, K. J.; Hegelich, B. M.

    2011-06-15

    Kinetic simulations of break-out-afterburner (BOA) ion acceleration from nm-scale targets are examined in a longer pulse length regime than studied previously. It is shown that when the target becomes relativistically transparent to the laser, an epoch of dramatic acceleration of ions occurs that lasts until the electron density in the expanding target reduces to the critical density in the non-relativistic limit. For given laser parameters, the optimal target thickness yielding the highest maximum ion energy is one in which this time window for ion acceleration overlaps with the intensity peak of the laser pulse. A simple analytic model of relativistically induced transparency is presented for plasma expansion at the time-evolving sound speed, from which these times may be estimated. The maximum ion energy attainable is controlled by the finite acceleration volume and time over which the BOA acts.

  6. Break-out afterburner ion acceleration in the longer laser pulse length regime

    NASA Astrophysics Data System (ADS)

    Yin, L.; Albright, B. J.; Jung, D.; Shah, R. C.; Palaniyappan, S.; Bowers, K. J.; Henig, A.; Fern´ndez, J. C.; Hegelich, B. M.

    2011-06-01

    Kinetic simulations of break-out-afterburner (BOA) ion acceleration from nm-scale targets are examined in a longer pulse length regime than studied previously. It is shown that when the target becomes relativistically transparent to the laser, an epoch of dramatic acceleration of ions occurs that lasts until the electron density in the expanding target reduces to the critical density in the non-relativistic limit. For given laser parameters, the optimal target thickness yielding the highest maximum ion energy is one in which this time window for ion acceleration overlaps with the intensity peak of the laser pulse. A simple analytic model of relativistically induced transparency is presented for plasma expansion at the time-evolving sound speed, from which these times may be estimated. The maximum ion energy attainable is controlled by the finite acceleration volume and time over which the BOA acts.

  7. Efficient quasi-monoenergetic ion beams from laser-driven relativistic plasmas

    DOE PAGES

    Palaniyappan, Sasi; Huang, Chengkun; Gautier, Donald C.; Hamilton, Christopher E.; Santiago, Miguel A.; Kreuzer, Christian; Sefkow, Adam B.; Shah, Rahul C.; Fernández, Juan C.

    2015-12-11

    Table-top laser–plasma ion accelerators have many exciting applications, many of which require ion beams with simultaneous narrow energy spread and high conversion efficiency. However, achieving these requirements has been elusive. We report the experimental demonstration of laser-driven ion beams with narrow energy spread and energies up to 18 MeV per nucleon and ~5% conversion efficiency (that is 4 J out of 80-J laser). Using computer simulations we identify a self-organizing scheme that reduces the ion energy spread after the laser exits the plasma through persisting self-generated plasma electric (~1012 V m-1) and magnetic (~104 T) fields. Furthermore, these results contributemore » to the development of next generation compact accelerators suitable for many applications such as isochoric heating for ion-fast ignition and producing warm dense matter for basic science.« less

  8. The laser ion source trap for highest isobaric selectivity in online exotic isotope productiona)

    NASA Astrophysics Data System (ADS)

    Schwellnus, F.; Blaum, K.; Catherall, R.; Crepieux, B.; Fedosseev, V.; Gottwald, T.; Kluge, H.-J.; Marsh, B.; Mattolat, C.; Rothe, S.; Stora, T.; Wendt, K.

    2010-02-01

    The improvement in the performance of a conventional laser ion source in the laser ion source and trap (LIST) project is presented, which envisages installation of a repeller electrode and a linear Paul trap/ion guide structure. This approach promises highest isobaric purity and optimum temporal and spatial control of the radioactive ion beam produced at an online isotope separator facility. The functionality of the LIST was explored at the offline test separators of University of Mainz (UMz) and ISOLDE/CERN, using the UMz solid state laser system. Ionization efficiency and selectivity as well as time structure and transversal emittance of the produced ion beam was determined. Next step after complete characterization is the construction and installation of the radiation-hard final trap structure and its first online application.

  9. The laser ion source trap for highest isobaric selectivity in online exotic isotope production.

    PubMed

    Schwellnus, F; Blaum, K; Catherall, R; Crepieux, B; Fedosseev, V; Gottwald, T; Kluge, H-J; Marsh, B; Mattolat, C; Rothe, S; Stora, T; Wendt, K

    2010-02-01

    The improvement in the performance of a conventional laser ion source in the laser ion source and trap (LIST) project is presented, which envisages installation of a repeller electrode and a linear Paul trap/ion guide structure. This approach promises highest isobaric purity and optimum temporal and spatial control of the radioactive ion beam produced at an online isotope separator facility. The functionality of the LIST was explored at the offline test separators of University of Mainz (UMz) and ISOLDE/CERN, using the UMz solid state laser system. Ionization efficiency and selectivity as well as time structure and transversal emittance of the produced ion beam was determined. Next step after complete characterization is the construction and installation of the radiation-hard final trap structure and its first online application. PMID:20192370

  10. Efficient quasi-monoenergetic ion beams from laser-driven relativistic plasmas

    SciTech Connect

    Palaniyappan, Sasi; Huang, Chengkun; Gautier, Donald C.; Hamilton, Christopher E.; Santiago, Miguel A.; Kreuzer, Christian; Sefkow, Adam B.; Shah, Rahul C.; Fernández, Juan C.

    2015-12-11

    Table-top laser–plasma ion accelerators have many exciting applications, many of which require ion beams with simultaneous narrow energy spread and high conversion efficiency. However, achieving these requirements has been elusive. We report the experimental demonstration of laser-driven ion beams with narrow energy spread and energies up to 18 MeV per nucleon and ~5% conversion efficiency (that is 4 J out of 80-J laser). Using computer simulations we identify a self-organizing scheme that reduces the ion energy spread after the laser exits the plasma through persisting self-generated plasma electric (~1012 V m-1) and magnetic (~104 T) fields. Furthermore, these results contribute to the development of next generation compact accelerators suitable for many applications such as isochoric heating for ion-fast ignition and producing warm dense matter for basic science.

  11. Efficient quasi-monoenergetic ion beams from laser-driven relativistic plasmas

    PubMed Central

    Palaniyappan, Sasi; Huang, Chengkun; Gautier, Donald C.; Hamilton, Christopher E.; Santiago, Miguel A.; Kreuzer, Christian; Sefkow, Adam B.; Shah, Rahul C.; Fernández, Juan C.

    2015-01-01

    Table-top laser–plasma ion accelerators have many exciting applications, many of which require ion beams with simultaneous narrow energy spread and high conversion efficiency. However, achieving these requirements has been elusive. Here we report the experimental demonstration of laser-driven ion beams with narrow energy spread and energies up to 18 MeV per nucleon and ∼5% conversion efficiency (that is 4 J out of 80-J laser). Using computer simulations we identify a self-organizing scheme that reduces the ion energy spread after the laser exits the plasma through persisting self-generated plasma electric (∼1012 V m−1) and magnetic (∼104 T) fields. These results contribute to the development of next generation compact accelerators suitable for many applications such as isochoric heating for ion-fast ignition and producing warm dense matter for basic science. PMID:26657147

  12. Ion response to relativistic electron bunches in the blowout regime of laser-plasma accelerators.

    PubMed

    Popov, K I; Rozmus, W; Bychenkov, V Yu; Naseri, N; Capjack, C E; Brantov, A V

    2010-11-01

    The ion response to relativistic electron bunches in the so called bubble or blowout regime of a laser-plasma accelerator is discussed. In response to the strong fields of the accelerated electrons the ions form a central filament along the laser axis that can be compressed to densities 2 orders of magnitude higher than the initial particle density. A theory of the filament formation and a model of ion self-compression are proposed. It is also shown that in the case of a sharp rear plasma-vacuum interface the ions can be accelerated by a combination of three basic mechanisms. The long time ion evolution that results from the strong electrostatic fields of an electron bunch provides a unique diagnostic of laser-plasma accelerators.

  13. Monoenergetic and GeV ion acceleration from the laser breakout afterburner using ultrathin targets

    SciTech Connect

    Yin, L.; Albright, B. J.; Hegelich, B. M.; Bowers, K. J.; Flippo, K. A.; Kwan, T. J. T.; Fernandez, J. C.

    2007-05-15

    A new laser-driven ion acceleration mechanism using ultrathin targets has been identified from particle-in-cell simulations. After a brief period of target normal sheath acceleration (TNSA) [S. P. Hatchett et al., Phys. Plasmas 7, 2076 (2000)], two distinct stages follow: first, a period of enhanced TNSA during which the cold electron background converts entirely to hot electrons, and second, the ''laser breakout afterburner'' (BOA) when the laser penetrates to the rear of the target where a localized longitudinal electric field is generated with the location of the peak field co-moving with the ions. During this process, a relativistic electron beam is produced by the ponderomotive drive of the laser. This beam is unstable to a relativistic Buneman instability, which rapidly converts the electron energy into ion energy. This mechanism accelerates ions to much higher energies using laser intensities comparable to earlier TNSA experiments. At a laser intensity of 10{sup 21} W/cm{sup 2}, the carbon ions accelerate as a quasimonoenergetic bunch to 100 s of MeV in the early stages of the BOA with conversion efficiency of order a few percent. Both are an order of magnitude higher than those realized from TNSA in recent experiments [Hegelich et al., Nature 441, 439 (2006)]. The laser-plasma interaction then evolves to produce a quasithermal energy distribution with maximum energy of {approx}2 GeV.

  14. An Integrated Microfabricated Device for Dual Microdialysis and On-line ESI Ion Trap Mass Spectrometry for the Analysis of Complex Biological Samples

    SciTech Connect

    Xiang, Fan; Lin, Yuehe ); Wen, Jian Y.; Matson, Dean W. ); Smith, Richard D. )

    1999-05-01

    A microfabricated dual-microdialysis device in a single integrated microfabricated platform was constructed using laser micromachining techniques for the rapid fractionation and cleanup of complex biological samples. Results suggest the potential for integration of such microfabricated devices with other sample manipulations for the rapid ESI-MS analysis of complex biological samples.

  15. Infrared ion spectroscopy in a modified quadrupole ion trap mass spectrometer at the FELIX free electron laser laboratory

    NASA Astrophysics Data System (ADS)

    Martens, Jonathan; Berden, Giel; Gebhardt, Christoph R.; Oomens, Jos

    2016-10-01

    We report on modifications made to a Paul-type quadrupole ion trap mass spectrometer and discuss its application in infrared ion spectroscopy experiments. Main modifications involve optical access to the trapped ions and hardware and software coupling to a variety of infrared laser sources at the FELIX infrared free electron laser laboratory. In comparison to previously described infrared ion spectroscopy experiments at the FELIX laboratory, we find significant improvements in efficiency and sensitivity. Effects of the trapping conditions of the ions on the IR multiple photon dissociation spectra are explored. Enhanced photo-dissociation is found at lower pressures in the ion trap. Spectra obtained under reduced pressure conditions are found to more closely mimic those obtained in the high-vacuum conditions of an Fourier transform ion cyclotron resonance mass spectrometer. A gas-mixing system is described enabling the controlled addition of a secondary gas into helium buffer gas flowing into the trap and allows for ion/molecule reactions in the trap. The electron transfer dissociation (ETD) option of the mass spectrometer allows for IR structure characterization of ETD-generated peptide dissociation products.

  16. Advances in surface ion suppression from RILIS: Towards the Time-of-Flight Laser Ion Source (ToF-LIS)

    NASA Astrophysics Data System (ADS)

    Rothe, S.; Catherall, R.; Crepieux, B.; Day Goodacre, T.; Fedosseev, V. N.; Giles, T.; Marsh, B. A.; Ramos, J. P.; Rossel, R. E.

    2016-06-01

    We present results from the development towards the Time-of-Flight Laser Ion Source (ToF-LIS) aiming for the suppression of isobaric contaminants through fast beam gating. The capability to characterize high resistance ion sources has been successfully demonstrated. A ninefold selectivity gain has been achieved through suppression of surface ionized potassium, while maintaining >90% transmission for laser-ionized gallium using a thin wall graphite ionizer cavity combined with a fast beam gate. Initial results from the investigation of glassy carbon as a potential hot cavity ion source are presented. Power-cycle tests of a newly designed mount for fragile ion source cavities indicates its capability to survive the thermal stress expected during operation in an ISOLDE target unit. Finally, we introduce fast ion beam switching at a rate of 10 kHz using the ISOLDE ion beam switchyard as a new concept for ion beam distribution and conclude by highlighting the potential applications of this ion beam multiplexing technique.

  17. Laser-induced fluorescence measurements of argon and xenon ion velocities near the sheath boundary in 3 ion species plasmas

    NASA Astrophysics Data System (ADS)

    Yip, Chi-Shung; Hershkowitz, Noah; Severn, Greg; Baalrud, Scott D.

    2016-05-01

    The Bohm sheath criterion is studied with laser-induced fluorescence in three ion species plasmas using two tunable diode lasers. Krypton is added to a low pressure unmagnetized DC hot filament discharge in a mixture of argon and xenon gas confined by surface multi-dipole magnetic fields. The argon and xenon ion velocity distribution functions are measured at the sheath-presheath boundary near a negatively biased boundary plate. The potential structures of the plasma sheath and presheath are measured by an emissive probe. Results are compared with previous experiments with Ar-Xe plasmas, where the two ion species were observed to reach the sheath edge at nearly the same speed. This speed was the ion sound speed of the system, which is consistent with the generalized Bohm criterion. In such two ion species plasmas, instability enhanced collisional friction was demonstrated [Hershkowitz et al., Phys. Plasmas 18(5), 057102 (2011).] to exist which accounted for the observed results. When three ion species are present, it is demonstrated under most circumstances the ions do not fall out of the plasma at their individual Bohm velocities. It is also shown that under most circumstances the ions do not fall out of the plasma at the system sound speed. These observations are also consistent with the presence of the instabilities.

  18. Ultra-relativistic ion acceleration in the laser-plasma interactions

    SciTech Connect

    Huang Yongsheng; Wang Naiyan; Tang Xiuzhang; Shi Yijin; Xueqing Yan

    2012-09-15

    An analytical relativistic model is proposed to describe the relativistic ion acceleration in the interaction of ultra-intense laser pulses with thin-foil plasmas. It is found that there is a critical value of the ion momentum to make sure that the ions are trapped by the light sail and accelerated in the radiation pressure acceleration (RPA) region. If the initial ion momentum is smaller than the critical value, that is in the classical case of RPA, the potential has a deep well and traps the ions to be accelerated, as the same described before by simulation results [Eliasson et al., New J. Phys. 11, 073006 (2009)]. There is a new ion acceleration region different from RPA, called ultra-relativistic acceleration, if the ion momentum exceeds the critical value. In this case, ions will experience a potential downhill. The dependence of the ion momentum and the self-similar variable at the ion front on the acceleration time has been obtained. In the ultra-relativistic limit, the ion momentum at the ion front is proportional to t{sup 4/5}, where t is the acceleration time. In our analytical hydrodynamical model, it is naturally predicted that the ion distribution from RPA is not monoenergetic, although the phase-stable acceleration mechanism is effective. The critical conditions of the laser and plasma parameters which identify the two acceleration modes have been achieved.

  19. Ridge waveguide lasers in Nd:GGG crystals produced by swift carbon ion irradiation and femtosecond laser ablation.

    PubMed

    Jia, Yuechen; Dong, Ningning; Chen, Feng; Vázquez de Aldana, Javier R; Akhmadaliev, Sh; Zhou, Shengqiang

    2012-04-23

    We report on the fabrication of ridge waveguide in Nd:GGG crystal by using swift C(5+) ion irradiation and femtosecond laser ablation. At room temperature continuous wave laser oscillation at wavelength of ~1063 nm has been realized through the optical pump at 808 nm with a slope efficiency of 41.8% and the pump threshold is 71.6 mW.

  20. Production of ultrahigh ion current densities at skin-layer subrelativistic laser plasma interaction

    NASA Astrophysics Data System (ADS)

    Badziak, J.; Glowacz, S.; Jablonski, S.; Parys, P.; Wolowski, J.; Hora, H.; Krása, J.; Láska, L.; Rohlena, K.

    2004-12-01

    Some applications of fast ions driven by a short (<=1 ps) laser pulse (e.g. fast ignition of ICF targets, x-ray laser pumping, laboratory astrophysics research or some nuclear physics experiments) require ion beams of picosecond (or shorter) time durations and of very high ion current densities (~1010 A cm-2 or higher). A possible way of producing ion beams with such extreme parameters is ballistic focusing of fast ions generated by a target normal sheath acceleration (TNSA) mechanism at relativistic laser intensities. In this paper we discuss another method, where the production of short-pulse ion beams of ultrahigh current densities is possible in a planar geometry at subrelativistic laser intensities and at a low energy (<=1 J) of the laser pulse. This method—referred to as skin-layer ponderomotive acceleration (S-LPA)—uses strong ponderomotive forces induced at the skin-layer interaction of a short laser pulse with a proper preplasma layer in front of a solid target. The basic features of the high-current ion generation by S-LPA were investigated using a simplified theory, numerical hydrodynamic simulations and measurements. The experiments were performed with subjoule 1 ps laser pulses interacting with massive or thin foil targets at intensities of up to 2 × 1017 W cm-2. It was found that both in the backward and forward directions highly collimated high-density ion beams (plasma blocks) with current densities at the ion source (close to the target) approaching 1010 A cm-2 are produced, in accordance with the theory and numerical calculations. These ion current densities were found to be comparable to (or even higher than) those estimated from recent short-pulse TNSA experiments with relativistic laser intensities. Apart from the simpler physics of the laser plasma interaction, the advantage of the considered method is the low energy of the driving laser pulses allowing the production of ultrahigh-current-density ion beams with a high repetition rate. It

  1. The influence of negative ions in helium-oxygen barrier discharges: I. Laser photodetachment experiment

    NASA Astrophysics Data System (ADS)

    Tschiersch, R.; Nemschokmichal, S.; Meichsner, J.

    2016-04-01

    This work is the experimental part of a comprehensive study that aims to understand the influence of negative ions on the development of atmospheric pressure barrier discharges in electronegative systems. The investigations will be complemented by a 1D numerical fluid simulation. Laser photodetachment experiments were performed in a glow-like barrier discharge operated in helium with admixtures of oxygen up to 1 vol.% at a gas pressure of 500 mbar. The discharge gap between the glass-coated electrodes was 3 mm. The discharge properties were characterized by electrical measurements and optical emission spectroscopy. Laser photodetachment of {{\\text{O}}-} , {\\text{O}}2- , and {\\text{O}}3- was studied using the fundamental and second harmonic wavelength of a Nd-YAG laser. The laser photodetachment of negative ions influences the breakdown characteristics when the laser is fired during the prephase of the discharge only. The breakdown voltage is reduced, which indicates an enhanced pre-ionization initiated by the detached electrons. Systematic variations in the laser pulse in time, the axial laser beam position, the laser pulse energy, and the laser wavelength provided detailed knowledge on this process. The investigation underlines the importance of the discharge prephase in general and aims to differentiate between the negative ion species {{\\text{O}}-} , {\\text{O}}2- , and {\\text{O}}3- .

  2. Polarization dependent fragmentation of ions produced by laser desorption from nanopost arrays.

    PubMed

    Stolee, Jessica A; Vertes, Akos

    2011-05-28

    Tailored silicon nanopost arrays (NAPA) enable controlled and resonant ion production in laser desorption ionization experiments and have been termed nanophotonic ion sources (Walker et al., J. Phys. Chem. C, 2010, 114, 4835-4840). As the post dimensions are comparable to or smaller than the laser wavelength, near-field effects and localized electromagnetic fields are present in their vicinity. In this contribution, we explore the desorption and ionization mechanism by studying how surface derivatization affects ion yields and fragmentation. We demonstrate that by increasing the laser fluence on derivatized NAPA with less polar surfaces that have decreased interaction energy between the structured silicon substrate and the adsorbate, the spectrum changes from exhibiting primarily molecular ions to showing a growing variety and abundance of fragments. The polarization angle of the laser beam had been shown to dramatically affect the ion yields of adsorbates. For the first time, we report that by rotating the plane of polarization of the desorption laser, the internal energy of the adsorbate can also be modulated resulting in polarization dependent fragmentation. This polarization effect also resulted in selective fragmentation of vitamin B(12). To explore the internal energy of NAPA generated ions, the effect of the post aspect ratios on the laser desorption thresholds and on the internal energy of a preformed ion was studied. Elevated surface temperatures and enhanced near fields in the vicinity of high aspect ratio posts are thought to contribute to desorption and ionization from NAPA. Comparison of the fluence dependence of the internal energies of ions produced from nanoporous silicon and NAPA substrates indicates that surface restructuring or transient melting by the desorption laser is a prerequisite for the former but not for the latter. PMID:21437297

  3. Polarization dependent fragmentation of ions produced by laser desorption from nanopost arrays.

    PubMed

    Stolee, Jessica A; Vertes, Akos

    2011-05-28

    Tailored silicon nanopost arrays (NAPA) enable controlled and resonant ion production in laser desorption ionization experiments and have been termed nanophotonic ion sources (Walker et al., J. Phys. Chem. C, 2010, 114, 4835-4840). As the post dimensions are comparable to or smaller than the laser wavelength, near-field effects and localized electromagnetic fields are present in their vicinity. In this contribution, we explore the desorption and ionization mechanism by studying how surface derivatization affects ion yields and fragmentation. We demonstrate that by increasing the laser fluence on derivatized NAPA with less polar surfaces that have decreased interaction energy between the structured silicon substrate and the adsorbate, the spectrum changes from exhibiting primarily molecular ions to showing a growing variety and abundance of fragments. The polarization angle of the laser beam had been shown to dramatically affect the ion yields of adsorbates. For the first time, we report that by rotating the plane of polarization of the desorption laser, the internal energy of the adsorbate can also be modulated resulting in polarization dependent fragmentation. This polarization effect also resulted in selective fragmentation of vitamin B(12). To explore the internal energy of NAPA generated ions, the effect of the post aspect ratios on the laser desorption thresholds and on the internal energy of a preformed ion was studied. Elevated surface temperatures and enhanced near fields in the vicinity of high aspect ratio posts are thought to contribute to desorption and ionization from NAPA. Comparison of the fluence dependence of the internal energies of ions produced from nanoporous silicon and NAPA substrates indicates that surface restructuring or transient melting by the desorption laser is a prerequisite for the former but not for the latter.

  4. The study towards high intensity high charge state laser ion sources.

    PubMed

    Zhao, H Y; Jin, Q Y; Sha, S; Zhang, J J; Li, Z M; Liu, W; Sun, L T; Zhang, X Z; Zhao, H W

    2014-02-01

    As one of the candidate ion sources for a planned project, the High Intensity heavy-ion Accelerator Facility, a laser ion source has been being intensively studied at the Institute of Modern Physics in the past two years. The charge state distributions of ions produced by irradiating a pulsed 3 J/8 ns Nd:YAG laser on solid targets of a wide range of elements (C, Al, Ti, Ni, Ag, Ta, and Pb) were measured with an electrostatic ion analyzer spectrometer, which indicates that highly charged ions could be generated from low-to-medium mass elements with the present laser system, while the charge state distributions for high mass elements were relatively low. The shot-to-shot stability of ion pulses was monitored with a Faraday cup for carbon target. The fluctuations within ±2.5% for the peak current and total charge and ±6% for pulse duration were demonstrated with the present setup of the laser ion source, the suppression of which is still possible.

  5. The study towards high intensity high charge state laser ion sources.

    PubMed

    Zhao, H Y; Jin, Q Y; Sha, S; Zhang, J J; Li, Z M; Liu, W; Sun, L T; Zhang, X Z; Zhao, H W

    2014-02-01

    As one of the candidate ion sources for a planned project, the High Intensity heavy-ion Accelerator Facility, a laser ion source has been being intensively studied at the Institute of Modern Physics in the past two years. The charge state distributions of ions produced by irradiating a pulsed 3 J/8 ns Nd:YAG laser on solid targets of a wide range of elements (C, Al, Ti, Ni, Ag, Ta, and Pb) were measured with an electrostatic ion analyzer spectrometer, which indicates that highly charged ions could be generated from low-to-medium mass elements with the present laser system, while the charge state distributions for high mass elements were relatively low. The shot-to-shot stability of ion pulses was monitored with a Faraday cup for carbon target. The fluctuations within ±2.5% for the peak current and total charge and ±6% for pulse duration were demonstrated with the present setup of the laser ion source, the suppression of which is still possible. PMID:24593615

  6. Experimental study of the dynamics of a ruby laser pumped by a CW argon-ion laser

    NASA Technical Reports Server (NTRS)

    Afzal, R. S.; Lin, W. P.; Lawandy, N. M.

    1989-01-01

    A study of the dynamics of a ruby laser pumped by a CW argon-ion laser is presented. The ruby laser is predominantly stable but has two accessible unstable states. One state exhibits chaotic output, while the other results in regular self-pulsing. The conditions needed for instability are discussed and homodyne spectra and temporal maps of the phase-space attractors are obtained. In addition, a numerical simulation of nonlinear beam propagation in ruby is presented that shows that strong deviations from plane-wave behavior exist, and that transverse effects must be incorporated into theoretical models of the instability.

  7. Development of a gas cell-based laser ion source for RIKEN PALIS

    NASA Astrophysics Data System (ADS)

    Sonoda, T.; Wada, M.; Tomita, H.; Sakamoto, C.; Takatsuka, T.; Noto, T.; Iimura, H.; Matsuo, Y.; Kubo, T.; Shinozuka, T.; Wakui, T.; Mita, H.; Naimi, S.; Furukawa, T.; Itou, Y.; Schury, P.; Miyatake, H.; Jeong, S.; Ishiyama, H.; Watanabe, Y.; Hirayama, Y.

    2013-04-01

    We developed a prototype laser ionization gas cell with a beam extraction system. This device is for use of PArasitic Laser Ion-Source (PALIS), which will be implemented into RIKEN's fragment separator, BigRIPS as a part of SLOWRI. Off-line resonant laser ionization for stable Co, Cu, Fe, Ni, Ti, Nb, Sn, In and Pd inside the gas cell, ion extraction and transport to the high-vacuum region via SPIG and QMS have been confirmed (Sonoda et al, Nucl Instrum Meth B 295:1, 2013).

  8. Stochastic ion heating from many overlapping laser beams in fusion plasmas.

    PubMed

    Michel, P; Rozmus, W; Williams, E A; Divol, L; Berger, R L; Town, R P J; Glenzer, S H; Callahan, D A

    2012-11-01

    In this Letter, we show through numerical simulations and analytical results that overlapping multiple (N) laser beams in plasmas can lead to strong stochastic ion heating from many (~N(2)) electrostatic perturbations driven by beat waves between pairs of laser beams. For conditions typical of inertial-confinement-fusion experiment conditions, hundreds of such beat waves are driven in mm(3)-scale plasmas, leading to ion heating rates of several keV/ns. This mechanism saturates cross-beam energy transfer, with a reduction of linear gains by a factor ~4-5 and can strongly modify the overall hydrodynamics evolution of such laser-plasma systems. PMID:23215392

  9. Production of fullerene ions by combining of plasma sputtering with laser ablation

    SciTech Connect

    Yamada, K. Saitoh, Y.; Yokota, W.

    2014-02-15

    We have produced C{sub 60} ion beams by combining plasma sputtering and laser ablation. A C{sub 60} sample was placed in an electron cyclotron resonance type ion source, negatively biased and sputtered by argon plasma. The beam current of C{sub 60}{sup +} decreased rapidly, but it was transiently recovered by a single laser shot that ablates the thin sample surface on the sputtered area. Temporal variations in beam current are reported in response to laser shots repeated at intervals of a few minutes.

  10. Mono-energetic ions emission by nanosecond laser solid target irradiation

    NASA Astrophysics Data System (ADS)

    Muoio, A.; Tudisco, S.; Altana, C.; Lanzalone, G.; Mascali, D.; Cirrone, G. A. P.; Schillaci, F.; Trifirò, A.

    2016-09-01

    An experimental campaign aiming to investigate the acceleration mechanisms through laser-matter interaction in nanosecond domain has been carried out at the LENS (Laser Energy for Nuclear Science) laboratory of INFN-LNS, Catania. Pure Al targets were irradiated by 6 ns laser pulses at different pumping energies, up to 2 J. Advanced diagnostics tools were used to characterize the plasma plume and ion production. We show the preliminary results of this experimental campaign, and especially the ones showing the production of multicharged ions having very narrow energy spreads.

  11. Radiation-Pressure Acceleration of Ion Beams Driven by Circularly Polarized Laser Pulses

    SciTech Connect

    Henig, A.; Hoerlein, R.; Kiefer, D.; Jung, D.; Habs, D.; Steinke, S.; Schnuerer, M.; Sokollik, T.; Nickles, P. V.; Sandner, W.; Schreiber, J.; Hegelich, B. M.; Yan, X. Q.; Meyer-ter-Vehn, J.; Tajima, T.

    2009-12-11

    We present experimental studies on ion acceleration from ultrathin diamondlike carbon foils irradiated by ultrahigh contrast laser pulses of energy 0.7 J focused to peak intensities of 5x10{sup 19} W/cm{sup 2}. A reduction in electron heating is observed when the laser polarization is changed from linear to circular, leading to a pronounced peak in the fully ionized carbon spectrum at the optimum foil thickness of 5.3 nm. Two-dimensional particle-in-cell simulations reveal that those C{sup 6+} ions are for the first time dominantly accelerated in a phase-stable way by the laser radiation pressure.

  12. Ion acceleration in shell cylinders irradiated by a short intense laser pulse

    SciTech Connect

    Andreev, A.; Platonov, K.; Sharma, A.; Murakami, M.

    2015-09-15

    The interaction of a short high intensity laser pulse with homo and heterogeneous shell cylinders has been analyzed using particle-in-cell simulations and analytical modeling. We show that the shell cylinder is proficient of accelerating and focusing ions in a narrow region. In the case of shell cylinder, the ion energy exceeds the ion energy for a flat target of the same thickness. The constructed model enables the evaluation of the ion energy and the number of ions in the focusing region.

  13. Ion acceleration in shell cylinders irradiated by a short intense laser pulse

    NASA Astrophysics Data System (ADS)

    Andreev, A.; Platonov, K.; Sharma, A.; Murakami, M.

    2015-09-01

    The interaction of a short high intensity laser pulse with homo and heterogeneous shell cylinders has been analyzed using particle-in-cell simulations and analytical modeling. We show that the shell cylinder is proficient of accelerating and focusing ions in a narrow region. In the case of shell cylinder, the ion energy exceeds the ion energy for a flat target of the same thickness. The constructed model enables the evaluation of the ion energy and the number of ions in the focusing region.

  14. In situ measurement of ions parameters of laser produced ion source using high resolution Thomson Parabola Spectrometer

    NASA Astrophysics Data System (ADS)

    Chaurasia, S.; Kaur, C.; Rastogi, V.; Poswal, A. K.; Munda, D. S.; Bhatia, R. K.; Nataraju, V.

    2016-08-01

    The laser produced plasma based heavy ion source has become an outstanding front end for heavy ion accelerators. Before being implemented in the heavy ion accelerators its detailed characterization is required. For this purpose, a high resolution and high dispersion Thomson parabola spectrometer comprising of Time-of-Flight diagnostics has been developed for the characterization of ions with energy in the range from 1 keV to 1 MeV/nucleon and incorporated in the Laser plasma experimental chamber. The ion spectrometer is optimized with graphite target. The carbon ions of charge states C1+ to C6+ are observed in the energy range from 3 keV to 300 keV, which has also been verified by Time-of-Flight measurement. Experimental results were matched with simulation done by SIMION 7.0 code which is used for the design of the spectrometer. We also developed data analysis software using Python language to measure in situ ion's parameters and the results are in better agreement to the experimental results than the commercially available software SIMION 7.0. The resolution of the spectrometer is ΔE/E = 0.026 @ 31 keV for charge state (C4+) of carbon.

  15. Extending the applicability of an open-ring trap to perform experiments with a single laser-cooled ion.

    PubMed

    Cornejo, J M; Colombano, M; Doménech, J; Block, M; Delahaye, P; Rodríguez, D

    2015-10-01

    A special ion trap was initially built up to perform β-ν correlation experiments with radioactive ions. The trap geometry is also well suited to perform experiments with laser-cooled ions, serving for the development of a new type of Penning trap, in the framework of the project TRAPSENSOR at the University of Granada. The goal of this project is to use a single (40)Ca(+) ion as detector for single-ion mass spectrometry. Within this project and without any modification to the initial electrode configuration, it was possible to perform Doppler cooling on (40)Ca(+) ions, starting from large clouds and reaching single ion sensitivity. This new feature of the trap might be important also for other experiments with ions produced at radioactive ion beam facilities. In this publication, the trap and the laser system will be described, together with their performance with respect to laser cooling applied to large ion clouds down to a single ion.

  16. Influence of charge exchange on the collection of the laser produced ions

    NASA Astrophysics Data System (ADS)

    Hasegawa, Shuichi; Takei, Manabu; Suzuki, Atsuyuki; Kurosawa, Hitoshi

    2001-12-01

    We evaluated influences of charge exchange on ion collection of laser isotope separation of uranium. We made a two-dimensional code based on fluid dynamics taking the charge exchange term into consideration. Parametric study was performed in terms of electric amplitude, ion density, and electron temperature. In addition to parallel electrode arrangement, calculations were performed for Π- and M-type arrangements. The ratio of charge exchanged ions is found to largely depend on the collection time.

  17. 2D electron density profile measurement in tokamak by laser-accelerated ion-beam probea)

    NASA Astrophysics Data System (ADS)

    Chen, Y. H.; Yang, X. Y.; Lin, C.; Wang, L.; Xu, M.; Wang, X. G.; Xiao, C. J.

    2014-11-01

    A new concept of Heavy Ion Beam Probe (HIBP) diagnostic has been proposed, of which the key is to replace the electrostatic accelerator of traditional HIBP by a laser-driven ion accelerator. Due to the large energy spread of ions, the laser-accelerated HIBP can measure the two-dimensional (2D) electron density profile of tokamak plasma. In a preliminary simulation, a 2D density profile was reconstructed with a spatial resolution of about 2 cm, and with the error below 15% in the core region. Diagnostics of 2D density fluctuation is also discussed.

  18. 2D electron density profile measurement in tokamak by laser-accelerated ion-beam probe.

    PubMed

    Chen, Y H; Yang, X Y; Lin, C; Wang, L; Xu, M; Wang, X G; Xiao, C J

    2014-11-01

    A new concept of Heavy Ion Beam Probe (HIBP) diagnostic has been proposed, of which the key is to replace the electrostatic accelerator of traditional HIBP by a laser-driven ion accelerator. Due to the large energy spread of ions, the laser-accelerated HIBP can measure the two-dimensional (2D) electron density profile of tokamak plasma. In a preliminary simulation, a 2D density profile was reconstructed with a spatial resolution of about 2 cm, and with the error below 15% in the core region. Diagnostics of 2D density fluctuation is also discussed.

  19. MeV negative ion generation from ultra-intense laser interaction with a water spray

    SciTech Connect

    Ter-Avetisyan, S.; Ramakrishna, B.; Borghesi, M.; Doria, D.; Zepf, M.; Sarri, G.; Ehrentraut, L.; Steinke, S.; Sandner, W.; Schnuerer, M.; Andreev, A.; Nickles, P. V.; Tikhonchuk, V.

    2011-08-01

    MeV negative oxygen ions are obtained from a water spray target irradiated by high intensity (5 x 10{sup 19} W/cm{sup 2}) and ultrashort (50 fs) laser pulses. Generation of negative ions is ascribed to electron-capture processes that the laser-accelerated high-energy positive ion experiences when it interacts with atoms in the spray. This mechanism implies the existence of a large number of MeV neutral oxygen atoms, which is consistent with indirect experimental evidence.

  20. MeV negative ion source from ultra-intense laser-matter interaction

    SciTech Connect

    Ter-Avetisyan, S.; Ramakrishna, B.; Doria, D.; Prasad, R.; Borghesi, M.; Andreev, A. A.; Steinke, S.; Schnuerer, M.; Nickles, P. V.; Tikhonchuk, V.

    2012-02-15

    Experimental demonstration of negative ion acceleration to MeV energies from sub-micron size droplets of water spray irradiated by ultra-intense laser pulses is presented. Thanks to the specific target configuration and laser parameters, more than 10{sup 9} negative ions per steradian solid angle in 5% energy bandwidth are accelerated in a stable and reliable manner. To our knowledge, by virtue of the ultra-short duration of the emission, this is by far the brightest negative ion source reported. The data also indicate the existence of beams of neutrals with at least similar numbers and energies.

  1. 2D electron density profile measurement in tokamak by laser-accelerated ion-beam probe

    SciTech Connect

    Chen, Y. H.; Yang, X. Y.; Lin, C. E-mail: cjxiao@pku.edu.cn; Wang, X. G.; Xiao, C. J. E-mail: cjxiao@pku.edu.cn; Wang, L.; Xu, M.

    2014-11-15

    A new concept of Heavy Ion Beam Probe (HIBP) diagnostic has been proposed, of which the key is to replace the electrostatic accelerator of traditional HIBP by a laser-driven ion accelerator. Due to the large energy spread of ions, the laser-accelerated HIBP can measure the two-dimensional (2D) electron density profile of tokamak plasma. In a preliminary simulation, a 2D density profile was reconstructed with a spatial resolution of about 2 cm, and with the error below 15% in the core region. Diagnostics of 2D density fluctuation is also discussed.

  2. Optimizing conversion efficiency and reducing ion energy in a laser-produced Gd plasma

    SciTech Connect

    Cummins, Thomas; Li Bowen; O'Gorman, Colm; Dunne, Padraig; Sokell, Emma; O'Sullivan, Gerry; Otsuka, Takamitsu; Yugami, Noboru; Higashiguchi, Takeshi; Jiang Weihua; Endo, Akira

    2012-02-06

    We have demonstrated an efficient extreme ultraviolet (EUV) source at 6.7 nm by irradiating Gd targets with 0.8 and 1.06 {mu}m laser pulses of 140 fs to 10 ns duration. Maximum conversion efficiency of 0.4% was observed within a 0.6% bandwidth. A Faraday cup observed ion yield and time of flight signals for ions from plasmas generated by each laser. Ion kinetic energy was lower for shorter pulse durations, which yielded higher electron temperatures required for efficient EUV emission, due to higher laser intensity. Picosecond laser pulses were found to be the best suited to 6.7 nm EUV source generation.

  3. Features in the ion emission of Cu, Al, and C plasmas produced by ultrafast laser ablation

    NASA Astrophysics Data System (ADS)

    Kelly, T. J.; Butler, T.; Walsh, N.; Hayden, P.; Costello, J. T.

    2015-12-01

    The bi-modal nature of charge integrated ion kinetic energy distributions, which result from ultrafast laser produced plasmas, is discussed in this paper. A negatively biased Faraday cup was used as a charge collector to measure ion distributions from three different solid targets that had been irradiated with an ultrafast laser in the fluence range 0.1 -1 J/cm 2 . A bi-modal time of flight distribution is found for all three targets (C, Al, and Cu). In the case of the metallic targets (Al and Cu), high- and low-kinetic energy peaks exhibit quite different dependencies on laser fluence, whereas for the semi-metallic target (C), both peaks scale similarly with ultrafast laser fluence. The results are discussed within the framework of a one dimensional capacitor model resulting in ion acceleration.

  4. Electron, Photon, and Ion Beams from the Relativistic Interaction of Petawatt Laser Pulses with Solid Targets

    SciTech Connect

    Hatchett, S.P.; Brown, C.G.; Cowan, T.E.; Henry, E.A.; Johnson, J.; Key, M.H.; Koch, J.A.; Langdon, A.B.; Lasinski, B.F.; Lee, R.W.; Mackinnon, A.J.; Pennington, D.M.; Perry, M.D.; Phillips, T.W.; Roth, M.; Sangster, T.C.; Singh, M.S.; Snavely, R.A.; Stoyer, M.A.; Wilks, S.C.; Yasuike, K.

    1999-11-12

    In our Petawatt laser experiments several hundred joules of 1 {micro}m laser light in 0.5-5.0 ps pulses with intensities up to 3 x 10{sup 20}Wcm{sup -2} were incident on solid targets producing a strongly relativistic interaction. The energy content, spectra, and angular patterns of the photon, electron, and ion radiations were diagnosed in a number of ways, including several novel (to laser physics) nuclear activation techniques. From the beamed bremsstrahlung we infer that about 40-50% of the laser energy is converted to broadly beamed hot electrons. Their direction centroid varies from shot to shot, but the beam has a consistent width. Extraordinarily luminous ion beams almost precisely normal to the rear of various targets are seen--up to 3 x 10{sup 13} protons with kT{sub ion} {approx} several MeV representing {approx}6% of the laser energy. We observe ion energies up to at least 55 MeV. The ions appear to originate from the rear target surfaces. The edge of the ion beam is very sharp, and collimation increases with ion energy. At the highest energies, a narrow feature appears in the ion spectra, and the apparent size of the emitting spot is smaller than the full back surface area. Any ion emission from the front of the targets is much less than from the rear and is not sharply beamed. The hot electrons generate a Debye sheath with electrostatic fields of order MV per micron which apparently accelerate the ions.

  5. Dense blocks of energetic ions driven by multi-petawatt lasers

    NASA Astrophysics Data System (ADS)

    Weng, S. M.; Liu, M.; Sheng, Z. M.; Murakami, M.; Chen, M.; Yu, L. L.; Zhang, J.

    2016-02-01

    Laser-driven ion accelerators have the advantages of compact size, high density, and short bunch duration over conventional accelerators. Nevertheless, it is still challenging to simultaneously enhance the yield and quality of laser-driven ion beams for practical applications. Here we propose a scheme to address this challenge via the use of emerging multi-petawatt lasers and a density-modulated target. The density-modulated target permits its ions to be uniformly accelerated as a dense block by laser radiation pressure. In addition, the beam quality of the accelerated ions is remarkably improved by embedding the target in a thick enough substrate, which suppresses hot electron refluxing and thus alleviates plasma heating. Particle-in-cell simulations demonstrate that almost all ions in a solid-density plasma of a few microns can be uniformly accelerated to about 25% of the speed of light by a laser pulse at an intensity around 1022 W/cm2. The resulting dense block of energetic ions may drive fusion ignition and more generally create matter with unprecedented high energy density.

  6. Dense blocks of energetic ions driven by multi-petawatt lasers

    PubMed Central

    Weng, S. M.; Liu, M.; Sheng, Z. M.; Murakami, M.; Chen, M.; Yu, L. L.; Zhang, J.

    2016-01-01

    Laser-driven ion accelerators have the advantages of compact size, high density, and short bunch duration over conventional accelerators. Nevertheless, it is still challenging to simultaneously enhance the yield and quality of laser-driven ion beams for practical applications. Here we propose a scheme to address this challenge via the use of emerging multi-petawatt lasers and a density-modulated target. The density-modulated target permits its ions to be uniformly accelerated as a dense block by laser radiation pressure. In addition, the beam quality of the accelerated ions is remarkably improved by embedding the target in a thick enough substrate, which suppresses hot electron refluxing and thus alleviates plasma heating. Particle-in-cell simulations demonstrate that almost all ions in a solid-density plasma of a few microns can be uniformly accelerated to about 25% of the speed of light by a laser pulse at an intensity around 1022 W/cm2. The resulting dense block of energetic ions may drive fusion ignition and more generally create matter with unprecedented high energy density. PMID:26924793

  7. Dense blocks of energetic ions driven by multi-petawatt lasers.

    PubMed

    Weng, S M; Liu, M; Sheng, Z M; Murakami, M; Chen, M; Yu, L L; Zhang, J

    2016-01-01

    Laser-driven ion accelerators have the advantages of compact size, high density, and short bunch duration over conventional accelerators. Nevertheless, it is still challenging to simultaneously enhance the yield and quality of laser-driven ion beams for practical applications. Here we propose a scheme to address this challenge via the use of emerging multi-petawatt lasers and a density-modulated target. The density-modulated target permits its ions to be uniformly accelerated as a dense block by laser radiation pressure. In addition, the beam quality of the accelerated ions is remarkably improved by embedding the target in a thick enough substrate, which suppresses hot electron refluxing and thus alleviates plasma heating. Particle-in-cell simulations demonstrate that almost all ions in a solid-density plasma of a few microns can be uniformly accelerated to about 25% of the speed of light by a laser pulse at an intensity around 10(22) W/cm(2). The resulting dense block of energetic ions may drive fusion ignition and more generally create matter with unprecedented high energy density. PMID:26924793

  8. Indirect determination of trace amounts of fluoride in natural waters by ion chromatography: a comparison of on-line post-column fluorimetry and ICP-MS detectors.

    PubMed

    Bayón, M M; Rodríguez Garcia, A; García Alonso, J I; Sanz-Medel, A

    1999-01-01

    An alternative method for the determination of trace levels of fluoride in drinking and sea-water samples is presented. It is based on the formation of the aluminium monofluoride complex in excess of Al3+ and separation of the two species formed (AlF2+ and Al3+) in a small (5 cm long, CG2) ion exchange guard column. The final determination is accomplished by both ICP-MS specific detection and post column derivatisation with fluorimetric detection. Fundamental studies on the formation kinetics of the complex, ion chromatographic separation and optimum aluminium concentration were carried out using spectrofluorimetric detection by post-column reaction of the species with 8-hydroxyquinoline-5-sulfonic acid in a micellar medium of cetyltrimethylammonium bromide. Fluorimetric detection showed good detection limits, but interferences from cations such as Mg2+ and Zn2+ required the use of the longer CS2 ion exchange column. Iron interfered in relatively large amounts but adding EDTA to the sample solution eliminated the interference. A similar separation methodology was applied using ICP-MS detection for the indirect determination of fluoride, by monitoring aluminium at mass 27. In this case, a detection limit of 0.1 ng ml-1 was obtained using 0.45 M HNO3 as eluent and no interference caused by high concentrations of iron was observed. The proposed method was applied to the determination of very low levels of fluoride in natural waters.

  9. Angular distribution of ions and extreme ultraviolet emission in laser-produced tin droplet plasma

    NASA Astrophysics Data System (ADS)

    Chen, Hong; Wang, Xinbing; Duan, Lian; Lan, Hui; Chen, Ziqi; Zuo, Duluo; Lu, Peixiang

    2015-05-01

    Angular-resolved ion time-of-flight spectra as well as extreme ultraviolet radiation in laser-produced tin droplet plasma are investigated experimentally and theoretically. Tin droplets with a diameter of 150 μm are irradiated by a pulsed Nd:YAG laser. The ion time-of-flight spectra measured from the plasma formed by laser irradiation of the tin droplets are interpreted in terms of a theoretical elliptical Druyvesteyn distribution to deduce ion density distributions including kinetic temperatures of the plasma. The opacity of the plasma for extreme ultraviolet radiation is calculated based on the deduced ion densities and temperatures, and the angular distribution of extreme ultraviolet radiation is expressed as a function of the opacity using the Beer-Lambert law. Our results show that the calculated angular distribution of extreme ultraviolet radiation is in satisfactory agreement with the experimental data.

  10. Proton and Ion Beams Generated with Picosecond CO{sub 2} Laser Pulses

    SciTech Connect

    Pogorelsky, Igor; Yakimenko, Vitaly; Stolyarov, Daniil; Shkolnikov, Peter; Chen Min; Pukhov, Alexander; McKenna, Paul; Carroll, David; Neely, David; Najmudin, Zulfikar; Willingale, Louise; Stolyarova, Elena; Flynn, George

    2009-01-22

    1-TW, 6-ps, circularly polarized CO{sub 2} laser pulses focused onto thin Al foils are used to drive ion acceleration. The spectra of ions and protons generated in the direction normal to the rear surface, detected with a compact magnet spectrometer with CR39, reveals a broad proton high-energy peak at {approx}1 MeV. This observation conforms to the theoretical predictions that circularly polarized laser pulses are less efficient than linearly polarized pulses in driving ion acceleration via the Target Normal Sheath Acceleration (TNSA) mechanism. Instead, there is evidence that the circularly polarized laser may provide direct ponderomotive acceleration of ions and protons. We report also the first application of the BNL proton source in nano-science. Irradiation of graphite and graphene films produced local defects and membranes for variety of applications.

  11. Angular distribution of ions and extreme ultraviolet emission in laser-produced tin droplet plasma

    SciTech Connect

    Chen, Hong; Duan, Lian; Lan, Hui; Wang, Xinbing Chen, Ziqi; Zuo, Duluo; Lu, Peixiang

    2015-05-21

    Angular-resolved ion time-of-flight spectra as well as extreme ultraviolet radiation in laser-produced tin droplet plasma are investigated experimentally and theoretically. Tin droplets with a diameter of 150 μm are irradiated by a pulsed Nd:YAG laser. The ion time-of-flight spectra measured from the plasma formed by laser irradiation of the tin droplets are interpreted in terms of a theoretical elliptical Druyvesteyn distribution to deduce ion density distributions including kinetic temperatures of the plasma. The opacity of the plasma for extreme ultraviolet radiation is calculated based on the deduced ion densities and temperatures, and the angular distribution of extreme ultraviolet radiation is expressed as a function of the opacity using the Beer–Lambert law. Our results show that the calculated angular distribution of extreme ultraviolet radiation is in satisfactory agreement with the experimental data.

  12. Highly Charged Ions from Laser-Cluster Interactions: Local-Field-Enhanced Impact Ionization and Frustrated Electron-Ion Recombination

    SciTech Connect

    Fennel, Thomas; Ramunno, Lora; Brabec, Thomas

    2007-12-07

    Our molecular dynamics analysis of Xe{sub 147-5083} clusters identifies two mechanisms that contribute to the yet unexplained observation of extremely highly charged ions in intense laser cluster experiments. First, electron impact ionization is enhanced by the local cluster electric field, increasing the highest charge states by up to 40%; a corresponding theoretical method is developed. Second, electron-ion recombination after the laser pulse is frustrated by acceleration electric fields typically used in ion detectors. This increases the highest charge states by up to 90%, as compared to the usual assumption of total recombination of all cluster-bound electrons. Both effects together augment the highest charge states by up to 120%, in reasonable agreement with experiments.

  13. Shot-to-shot reproducibility in the emission of fast highly charged metal ions from a laser ion source

    SciTech Connect

    Krasa, J.; Velyhan, A.; Margarone, D.; Krousky, E.; Laska, L.; Jungwirth, K.; Rohlena, K.; Ullschmied, J.; Parys, P.; Ryc, L.; Wolowski, J.

    2012-02-15

    The generation of fast highly charged metal ions with the use of the sub-nanosecond Prague Asterix Laser System, operated at a fundamental wavelength of 1315 nm, is reported. Particular attention is paid to shot-to-shot reproducibility in the ion emission. Au and Pd targets were exposed to intensities up to 5 x 10{sup 16} W/cm{sup 2}. Above the laser intensity threshold of {approx}3 x 10{sup 14} W/cm{sup 2} the plasma is generated in a form of irregular bursts. The maximum energy of protons constituting the leading edge of the fastest burst reaches a value up to 1 MeV. The fast ions in the following bursts have energy gradually decreasing with the increasing burst number, namely, from a value of about 0.5 MeV/charge regardless of the atomic number and mass of the ionized species.

  14. Enhancement of ion generation in femtosecond ultraintense laser-foil interactions by defocusing

    SciTech Connect

    Xu, M. H.; Li, Y. T.; Liu, F.; Carroll, D. C.; McKenna, P.; Foster, P. S.; Hawkes, S.; Streeter, M. J. V.; Spindloe, C.; Neely, D.; Kar, S.; Markey, K.; Zepf, M.; Sheng, Z. M.; Zhang, J.; Wahlstroem, C.-G.; Zheng, J.

    2012-02-20

    A simple method to enhance ion generation with femtosecond ultraintense lasers is demonstrated experimentally by defocusing laser beams on target surface. When the laser is optimally defocused, we find that the population of medium and low energy protons from ultra-thin foils is increased significantly while the proton cutoff energy is almost unchanged. In this way, the total proton yield can be enhanced by more than 1 order, even though the peak laser intensity drops. The depression of the amplified spontaneous emission (ASE) effect and the population increase of moderate-energy electrons are believed to be the main reasons for the effective enhancement.

  15. Formation of the characteristics of ion emission from a laser-produced plasma in the presence of a conducting diaphragm

    SciTech Connect

    Bykovskii, Yurii A; Konyukhov, I Yu; Peklenkov, V D; Ponomarenko, D V

    2000-08-31

    The effect of electrical diaphragm-target coupling on the formation of ion component characteristics of a laser-produced plasma is considered. When the target and the diaphragm are insulated from each other and are under a floating potential, a high-energy ion peak is observed and the integral number of ions and their multiplicity increase compared to the case when the target and the diaphragm are connected and grounded. (interaction of laser radiation with matter. laser plasma)

  16. Laser-based ion sources for medical applications

    NASA Astrophysics Data System (ADS)

    Bychenkov, V. Yu.; Brantov, A. V.

    2015-10-01

    Interaction of relativistic short laser pulses with thin foils is studied by using 3D PIC simulations in the context of ICAN's "dream laser". It is shown that such a laser will make it possible to accelerate protons and deuterons to multi-MeV energies with a current density of 100 A/cm2. The laser-triggered hadron beams may trigger nuclear reactions of interest for nuclear medicine and pharmacy. As an example, the yields C-11 for PET, of Tc-99m for SPECT, and neutrons for therapy have been analyzed.

  17. Motion of the plasma critical layer during relativistic-electron laser interaction with immobile and comoving ion plasma for ion acceleration

    SciTech Connect

    Sahai, Aakash A.

    2014-05-15

    We analyze the motion of the plasma critical layer by two different processes in the relativistic-electron laser-plasma interaction regime (a{sub 0}>1). The differences are highlighted when the critical layer ions are stationary in contrast to when they move with it. Controlling the speed of the plasma critical layer in this regime is essential for creating low-β traveling acceleration structures of sufficient laser-excited potential for laser ion accelerators. In Relativistically Induced Transparency Acceleration (RITA) scheme, the heavy plasma-ions are fixed and only trace-density light-ions are accelerated. The relativistic critical layer and the acceleration structure move longitudinally forward by laser inducing transparency through apparent relativistic increase in electron mass. In the Radiation Pressure Acceleration (RPA) scheme, the whole plasma is longitudinally pushed forward under the action of the laser radiation pressure, possible only when plasma ions co-propagate with the laser front. In RPA, the acceleration structure velocity critically depends upon plasma-ion mass in addition to the laser intensity and plasma density. In RITA, mass of the heavy immobile plasma-ions does not affect the speed of the critical layer. Inertia of the bared immobile ions in RITA excites the charge separation potential, whereas RPA is not possible when ions are stationary.

  18. Motion of the plasma critical layer during relativistic-electron laser interaction with immobile and comoving ion plasma for ion accelerationa)

    NASA Astrophysics Data System (ADS)

    Sahai, Aakash A.

    2014-05-01

    We analyze the motion of the plasma critical layer by two different processes in the relativistic-electron laser-plasma interaction regime (a0>1). The differences are highlighted when the critical layer ions are stationary in contrast to when they move with it. Controlling the speed of the plasma critical layer in this regime is essential for creating low-β traveling acceleration structures of sufficient laser-excited potential for laser ion accelerators. In Relativistically Induced Transparency Acceleration (RITA) scheme, the heavy plasma-ions are fixed and only trace-density light-ions are accelerated. The relativistic critical layer and the acceleration structure move longitudinally forward by laser inducing transparency through apparent relativistic increase in electron mass. In the Radiation Pressure Acceleration (RPA) scheme, the whole plasma is longitudinally pushed forward under the action of the laser radiation pressure, possible only when plasma ions co-propagate with the laser front. In RPA, the acceleration structure velocity critically depends upon plasma-ion mass in addition to the laser intensity and plasma density. In RITA, mass of the heavy immobile plasma-ions does not affect the speed of the critical layer. Inertia of the bared immobile ions in RITA excites the charge separation potential, whereas RPA is not possible when ions are stationary.

  19. Three-Dimensional Dynamics of Breakout Afterburner Ion Acceleration Using High-Contrast Short-Pulse Laser and Nanoscale Targets

    NASA Astrophysics Data System (ADS)

    Yin, L.; Albright, B. J.; Bowers, K. J.; Jung, D.; Fernández, J. C.; Hegelich, B. M.

    2011-07-01

    Breakout afterburner (BOA) laser-ion acceleration has been demonstrated for the first time in the laboratory. In the BOA, an initially solid-density target undergoes relativistically induced transparency, initiating a period of enhanced ion acceleration. First-ever kinetic simulations of the BOA in three dimensions show that the ion beam forms lobes in the direction orthogonal to laser polarization and propagation. Analytic theory presented for the electron dynamics in the laser ponderomotive field explains how azimuthal symmetry breaks even for a symmetric laser intensity profile; these results are consistent with recent experiments at the Trident laser facility.

  20. Three-dimensional dynamics of breakout afterburner ion acceleration using high-contrast short-pulse laser and nanoscale targets.

    PubMed

    Yin, L; Albright, B J; Bowers, K J; Jung, D; Fernández, J C; Hegelich, B M

    2011-07-22

    Breakout afterburner (BOA) laser-ion acceleration has been demonstrated for the first time in the laboratory. In the BOA, an initially solid-density target undergoes relativistically induced transparency, initiating a period of enhanced ion acceleration. First-ever kinetic simulations of the BOA in three dimensions show that the ion beam forms lobes in the direction orthogonal to laser polarization and propagation. Analytic theory presented for the electron dynamics in the laser ponderomotive field explains how azimuthal symmetry breaks even for a symmetric laser intensity profile; these results are consistent with recent experiments at the Trident laser facility.

  1. On-Line Cataloging.

    ERIC Educational Resources Information Center

    OCLC Online Computer Library Center, Inc., Dublin, OH.

    The principal objective of the Ohio College Library Center is to lower the rate of rise of per-unit library costs while increasing the availability of library resources for use by patrons of participating libraries. A major procedural goal of the on-line cataloging system is to furnish cataloging personnel in individual libraries with…

  2. A new direct laser photo-induced fluorescence method coupled on-line with liquid chromatographic separation for the simultaneous determination of anilides pesticides.

    PubMed

    Mbaye, O M A; Maroto, A; Gaye-Seye, M D; Stephan, L; Deschamps, L; Aaron, J J; Giamarchi, P

    2015-01-01

    A new direct laser photo-induced fluorescence high performance liquid chromatography (DL-PIF-HPLC) method is developed for the simultaneous determination of three anilide pesticides, namely carboxin, monalide and propanil. DL-PIF-HPLC uses a tunable Nd:YAG-OPO laser to obtain fluorescent photoproduct(s) and to simultaneously analyze their fluorescence in a short acquisition time with an intensified CCD camera, which improves the selectivity (by choosing the suitable excitation wavelength), increases the sensitivity (due to the high energy of the laser beam) and reduces the time of analysis, relative to the classical PIF methods. However, one of the main drawbacks of PIF methods is the presence of interferences with other compounds, such as other pesticides from the same group yielding similar fluorescent photoproducts, which reduces their selectivity. The analytical interest of DL-PIF-HPLC to avoid these interferences is demonstrated. The DL-PIF spectra, chromatographic conditions and analytical performances of DL-PIF-HPLC are presented for the simultaneous determination of three anilide pesticides. The calibration curves are linear over one order of magnitude and the limits of detection are in the ng mL(-1) range. The new DL-PIF-HPLC system has the advantage to combine the performances of both techniques, DL-PIF and liquid chromatography, and to improve the analysis selectivity. PMID:25476396

  3. A new direct laser photo-induced fluorescence method coupled on-line with liquid chromatographic separation for the simultaneous determination of anilides pesticides.

    PubMed

    Mbaye, O M A; Maroto, A; Gaye-Seye, M D; Stephan, L; Deschamps, L; Aaron, J J; Giamarchi, P

    2015-01-01

    A new direct laser photo-induced fluorescence high performance liquid chromatography (DL-PIF-HPLC) method is developed for the simultaneous determination of three anilide pesticides, namely carboxin, monalide and propanil. DL-PIF-HPLC uses a tunable Nd:YAG-OPO laser to obtain fluorescent photoproduct(s) and to simultaneously analyze their fluorescence in a short acquisition time with an intensified CCD camera, which improves the selectivity (by choosing the suitable excitation wavelength), increases the sensitivity (due to the high energy of the laser beam) and reduces the time of analysis, relative to the classical PIF methods. However, one of the main drawbacks of PIF methods is the presence of interferences with other compounds, such as other pesticides from the same group yielding similar fluorescent photoproducts, which reduces their selectivity. The analytical interest of DL-PIF-HPLC to avoid these interferences is demonstrated. The DL-PIF spectra, chromatographic conditions and analytical performances of DL-PIF-HPLC are presented for the simultaneous determination of three anilide pesticides. The calibration curves are linear over one order of magnitude and the limits of detection are in the ng mL(-1) range. The new DL-PIF-HPLC system has the advantage to combine the performances of both techniques, DL-PIF and liquid chromatography, and to improve the analysis selectivity.

  4. Femtosecond Laser-Induced Upconversion Luminescence in Rare-Earth Ions by Nonresonant Multiphoton Absorption.

    PubMed

    Yao, Yunhua; Xu, Cheng; Zheng, Ye; Yang, Chengshuai; Liu, Pei; Jia, Tianqing; Qiu, Jianrong; Sun, Zhenrong; Zhang, Shian

    2016-07-21

    The upconversion luminescence of rare-earth ions has attracted considerable interest because of its important applications in photoelectric conversion, color display, laser device, multiplexed biolabeling, and security printing. Previous studies mainly explored the upconversion luminescence generation through excited state absorption, energy transfer upconversion, and photon avalanche under the continuous wave laser excitation. Here, we focus on the upconversion luminescence generation through a nonresonant multiphoton absorption by using the intense femtosecond pulsed laser excitation and study the upconversion luminescence intensity control by varying the femtosecond laser phase and polarization. We show that the upconversion luminescence of rare-earth ions under the intense femtosecond laser field excitation is easy to be obtained due to the nonresonant multiphoton absorption through the nonlinear interaction between light and matter, which is not available by the continuous wave laser excitation in previous works. We also show that the upconversion luminescence intensity can be effectively controlled by varying the femtosecond pulsed laser phase and polarization, which can open a new technological opportunity to generate and control the upconversion luminescence of rare-earth ions and also can be further extended to the relevant application areas. PMID:27367751

  5. On the analysis of inhomogeneous magnetic field spectrometer for laser-driven ion acceleration

    SciTech Connect

    Jung, D.; Senje, L.; McCormack, O.; Dromey, B.; Zepf, M.; Yin, L.; Albright, B. J.; Letzring, S.; Gautier, D. C.; Fernandez, J. C.; Toncian, T.; Hegelich, B. M.

    2015-03-15

    We present a detailed study of the use of a non-parallel, inhomogeneous magnetic field spectrometer for the investigation of laser-accelerated ion beams. Employing a wedged yoke design, we demonstrate the feasibility of an in-situ self-calibration technique of the non-uniform magnetic field and show that high-precision measurements of ion energies are possible in a wide-angle configuration. We also discuss the implications of a stacked detector system for unambiguous identification of different ion species present in the ion beam and explore the feasibility of detection of high energy particles beyond 100 MeV/amu in radiation harsh environments.

  6. Ion acceleration in a solitary wave by an intense picosecond laser pulse.

    PubMed

    Zhidkov, A; Uesaka, M; Sasaki, A; Daido, H

    2002-11-18

    Acceleration of ions in a solitary wave produced by shock-wave decay in a plasma slab irradiated by an intense picosecond laser pulse is studied via particle-in-cell simulation. Instead of exponential distribution as in known mechanisms of ion acceleration from the target surface, these ions accelerated forwardly form a bunch with relatively low energy spread. The bunch is shown to be a solitary wave moving over expanding plasma; its velocity can exceed the maximal velocity of ions accelerated forward from the rear side of the target.

  7. In situ and on-line monitoring of CO in an industrial glass furnace by mid-infrared difference-frequency generation laser spectroscopy.

    PubMed

    Khorsandi, Alireza; Willer, Ulrike; Wondraczek, Lothar; Schade, Wolfgang

    2004-12-10

    A compact mid-infrared (MIR) laser spectrometer based on difference-frequency generation (DFG) is applied as a portable and sensitive gas sensor for industrial process control and pollutant monitoring. We demonstrate the performance of such a MIR DFG gas sensor by recording the absorption spectra of the carbon monoxide (CO) P(28) absorption line in the atmosphere of a gas-fired glass melting furnace. For a gas temperature of approximately 1100 degrees C, the CO concentration in the recuperator channel is measured to be 400 parts per million.

  8. Prospects for ultrafast lasers in ion-radiography

    SciTech Connect

    Nickles, P. V.; Schnuerer, M.; Steinke, S.; Sokollik, T.; Ter-Avetisyan, S.; Sandner, W.; Nakamura, T.; Mima, M.; Andreev, A.

    2008-06-24

    We demonstrate the feasibility of field mapping with proton beams having kinetic energies between 1-2 Megaelectronvolt. Adjustment of the ultrafast (40 fs) laser driven TNSA mechanism delivers a nearly pure proton beam with a low transversal emittance and an emerging broad kinetic spectrum. Suitable electronic image detection allows tracing of the temporal field evolution with temporal snapshots. An increase by a factor of more than 8 of the proton drive efficiency in terms of laser energy consumption has been achieved with thin foil targets (400 nm) when the temporal laser contrast was enhanced to 10 orders of magnitude by means of a double plasma mirror.

  9. Determination of trace metal ions via on-line separation and preconcentration by means of chelating Sepharose beads in a sequential injection lab-on-valve (SI-LOV) system coupled to electrothermal atomic absorption spectrometric detection.

    PubMed

    Long, Xiangbao; Hansen, Elo Harald; Miró, Manuel

    2005-06-15

    The analytical performance of an on-line sequential injection lab-on-valve (SI-LOV) system using chelating Sepharose beads as sorbent material for the determination of ultra-trace levels of Cd(II), Pb(II) and Ni(II) by electrothermal atomic absorption spectrometry (ETAAS) is described and discussed. The samples are adjusted to pH 5.0 on-line in the system for optimum operation. The target ions are adsorbed by chelation on the surface of the beads, contained in a 20mul microcolumn within the LOV, and following elution by 50mul 2M nitric acid, the eluate is, as sandwiched by air segments, introduced into the ETAAS. Based on the consumption of 1.8ml sample solution, retention efficiencies of 95, 75 and 90%, enrichment factors of 34, 27 and 32, and determination limits of 0.001, 0.07 and 0.02mugl(-1) were obtained for Cd(II), Pb(II) and Ni(II), respectively. The beads can be used repeatedly for at least 20 times without decrease of performance, yet can be replaced at will if the circumstances should so dictate. The optimized procedural parameters showed that 12 samples per hour could be prepared and successfully analyzed. The results obtained for three standard reference materials agreed very well with the certified values.

  10. Universal gate-set for trapped-ion qubits using a narrow linewidth diode laser

    NASA Astrophysics Data System (ADS)

    Akerman, Nitzan; Navon, Nir; Kotler, Shlomi; Glickman, Yinnon; Ozeri, Roee

    2015-11-01

    We report on the implementation of a high fidelity universal gate-set on optical qubits based on trapped 88Sr+ ions for the purpose of quantum information processing. All coherent operations were performed using a narrow linewidth diode laser. We employed a master-slave configuration for the laser, where an ultra low expansion glass Fabry-Perot cavity is used as a stable reference as well as a spectral filter. We characterized the laser spectrum using the ions with a modified Ramsey sequence which eliminated the affect of the magnetic field noise. We demonstrated high fidelity single qubit gates with individual addressing, based on inhomogeneous micromotion, on a two-ion chain as well as the Mølmer-Sørensen two-qubit entangling gate.

  11. A compact broadband ion beam focusing device based on laser-driven megagauss thermoelectric magnetic fields.

    PubMed

    Albertazzi, B; d'Humières, E; Lancia, L; Dervieux, V; Antici, P; Böcker, J; Bonlie, J; Breil, J; Cauble, B; Chen, S N; Feugeas, J L; Nakatsutsumi, M; Nicolaï, P; Romagnani, L; Shepherd, R; Sentoku, Y; Swantusch, M; Tikhonchuk, V T; Borghesi, M; Willi, O; Pépin, H; Fuchs, J

    2015-04-01

    Ultra-intense lasers can nowadays routinely accelerate kiloampere ion beams. These unique sources of particle beams could impact many societal (e.g., proton-therapy or fuel recycling) and fundamental (e.g., neutron probing) domains. However, this requires overcoming the beam angular divergence at the source. This has been attempted, either with large-scale conventional setups or with compact plasma techniques that however have the restriction of short (<1 mm) focusing distances or a chromatic behavior. Here, we show that exploiting laser-triggered, long-lasting (>50 ps), thermoelectric multi-megagauss surface magnetic (B)-fields, compact capturing, and focusing of a diverging laser-driven multi-MeV ion beam can be achieved over a wide range of ion energies in the limit of a 5° acceptance angle.

  12. A compact broadband ion beam focusing device based on laser-driven megagauss thermoelectric magnetic fields.

    PubMed

    Albertazzi, B; d'Humières, E; Lancia, L; Dervieux, V; Antici, P; Böcker, J; Bonlie, J; Breil, J; Cauble, B; Chen, S N; Feugeas, J L; Nakatsutsumi, M; Nicolaï, P; Romagnani, L; Shepherd, R; Sentoku, Y; Swantusch, M; Tikhonchuk, V T; Borghesi, M; Willi, O; Pépin, H; Fuchs, J

    2015-04-01

    Ultra-intense lasers can nowadays routinely accelerate kiloampere ion beams. These unique sources of particle beams could impact many societal (e.g., proton-therapy or fuel recycling) and fundamental (e.g., neutron probing) domains. However, this requires overcoming the beam angular divergence at the source. This has been attempted, either with large-scale conventional setups or with compact plasma techniques that however have the restriction of short (<1 mm) focusing distances or a chromatic behavior. Here, we show that exploiting laser-triggered, long-lasting (>50 ps), thermoelectric multi-megagauss surface magnetic (B)-fields, compact capturing, and focusing of a diverging laser-driven multi-MeV ion beam can be achieved over a wide range of ion energies in the limit of a 5° acceptance angle. PMID:25933857

  13. Complementary ion and extreme ultra-violet spectrometer for laser-plasma diagnosis

    SciTech Connect

    Ter-Avetisyan, S.; Ramakrishna, B.; Doria, D.; Sarri, G.; Zepf, M.; Borghesi, M.; Ehrentraut, L.; Stiel, H.; Steinke, S.; Schnuerer, M.; Nickles, P. V.; Sandner, W.; Priebe, G.

    2009-10-15

    Simultaneous detection of extreme ultra-violet (XUV) and ion emission along the same line of sight provides comprehensive insight into the evolution of plasmas. This type of combined spectroscopy is applied to diagnose laser interaction with a spray target. The use of a micro-channel-plate detector assures reliable detection of both XUV and ion signals in a single laser shot. The qualitative analysis of the ion emission and XUV spectra allows to gain detailed information about the plasma conditions, and a correlation between the energetic proton emission and the XUV plasma emission can be suggested. The measured XUV emission spectrum from water spray shows efficient deceleration of laser accelerated electrons with energies up to keV in the initially cold background plasma and the collisional heating of the plasma.

  14. A compact broadband ion beam focusing device based on laser-driven megagauss thermoelectric magnetic fields

    NASA Astrophysics Data System (ADS)

    Albertazzi, B.; d'Humières, E.; Lancia, L.; Dervieux, V.; Antici, P.; Böcker, J.; Bonlie, J.; Breil, J.; Cauble, B.; Chen, S. N.; Feugeas, J. L.; Nakatsutsumi, M.; Nicolaï, P.; Romagnani, L.; Shepherd, R.; Sentoku, Y.; Swantusch, M.; Tikhonchuk, V. T.; Borghesi, M.; Willi, O.; Pépin, H.; Fuchs, J.

    2015-04-01

    Ultra-intense lasers can nowadays routinely accelerate kiloampere ion beams. These unique sources of particle beams could impact many societal (e.g., proton-therapy or fuel recycling) and fundamental (e.g., neutron probing) domains. However, this requires overcoming the beam angular divergence at the source. This has been attempted, either with large-scale conventional setups or with compact plasma techniques that however have the restriction of short (<1 mm) focusing distances or a chromatic behavior. Here, we show that exploiting laser-triggered, long-lasting (>50 ps), thermoelectric multi-megagauss surface magnetic (B)-fields, compact capturing, and focusing of a diverging laser-driven multi-MeV ion beam can be achieved over a wide range of ion energies in the limit of a 5° acceptance angle.

  15. Spot size dependence of laser accelerated protons in thin multi-ion foils

    SciTech Connect

    Liu, Tung-Chang Shao, Xi; Liu, Chuan-Sheng; Eliasson, Bengt; Wang, Jyhpyng; Chen, Shih-Hung

    2014-06-15

    We present a numerical study of the effect of the laser spot size of a circularly polarized laser beam on the energy of quasi-monoenergetic protons in laser proton acceleration using a thin carbon-hydrogen foil. The used proton acceleration scheme is a combination of laser radiation pressure and shielded Coulomb repulsion due to the carbon ions. We observe that the spot size plays a crucial role in determining the net charge of the electron-shielded carbon ion foil and consequently the efficiency of proton acceleration. Using a laser pulse with fixed input energy and pulse length impinging on a carbon-hydrogen foil, a laser beam with smaller spot sizes can generate higher energy but fewer quasi-monoenergetic protons. We studied the scaling of the proton energy with respect to the laser spot size and obtained an optimal spot size for maximum proton energy flux. Using the optimal spot size, we can generate an 80 MeV quasi-monoenergetic proton beam containing more than 10{sup 8} protons using a laser beam with power 250 TW and energy 10 J and a target of thickness 0.15 wavelength and 49 critical density made of 90% carbon and 10% hydrogen.

  16. Investigating the Heating of a Potassium-Doped Aluminosilicate Ion Source Using a 1 Micron Laser

    SciTech Connect

    Schmitt, R C; Meier, W R; Kwan, J W; Abbott, R P; Latkowski, J F

    2004-12-14

    The heavy ion fusion (HIF) program is interested in developing a high brightness ion source for high energy density physics (HEDP) experiments. One possible approach to obtaining higher brightness may be to raise the surface temperature of the ion source just prior to extraction. The current ion source material being studied is a layer of potassium-doped aluminosilicate bonded to a tungsten substrate. It is speculated that if the surface temperature of the source is raised above 1200 C (from a steady-state temperature of 900 C) for time periods on the order of 100's of nanoseconds, current densities of greater than 100 mA/cm{sup 2} of ions may be achievable. Typical aluminosilicate sources produce ion current densities (either K+ or Na+ ions) of {approx}10 mA/cm{sup 2} (at 1100 C). A number of heating methods might be possible, including lasers, diode arrays, and flash lamps. Here we assume laser heating. In this preliminary study, we used the LLNL RadHeat code to model the time-temperature history of the surface when hit by laser pulses and illustrate how RadHeat can be used to optimize the surface temperature response. Also of interest is the temperature history of the interface temperature between the ceramic and the metal layers. This is also investigated.

  17. Kinetics of ion and prompt electron emission from laser-produced plasma

    SciTech Connect

    Farid, N.; Harilal, S. S.; Hassanein, A.; Ding, H.

    2013-07-15

    We investigated ion emission dynamics of laser-produced plasma from several elements, comprised of metals and non-metals (C, Al, Si, Cu, Mo, Ta, W), under vacuum conditions using a Faraday cup. The estimated ion flux for various targets studied showed a decreasing tendency with increasing atomic mass. For metals, the ion flux is found to be a function of sublimation energy. A comparison of temporal ion profiles of various materials showed only high-Z elements exhibited multiple structures in the ion time of flight profile indicated by the observation of higher peak kinetic energies, which were absent for low-Z element targets. The slower ions were seen regardless of the atomic number of target material propagated with a kinetic energy of 1–5 keV, while the fast ions observed in high-Z materials possessed significantly higher energies. A systematic study of plasma properties employing fast photography, time, and space resolved optical emission spectroscopy, and electron analysis showed that there existed different mechanisms for generating ions in laser ablation plumes. The origin of high kinetic energy ions is related to prompt electron emission from high-Z targets.

  18. DBR laser with nondynamic plasma grating formed by focused ion beam implanted dopants

    NASA Technical Reports Server (NTRS)

    Boenke, Myra M.; Wu, M. C.; Wang, Shyh; Clark, William M., Jr.; Stevens, Eugene H.

    1989-01-01

    A static plasma grating has been demonstrated experimentally (Wu et al., 1988) in a large-optical-cavity focused-ion-beam-distributed-Bragg-reflector (FIB-DBR) GaAlAs/GaAs laser diode. The grating is formed by implanting stripes of dopants with a focused ion beam. The dopants ionize to form periodic fluctuations in the carrier concentration which, through the Kramers-Kronig relations, form an index grating. A model of the grating strength for optimizaton of the laser design is developed and presented. The computed results show that the coupling coefficient k can be increased by more than an order of magnitude over the 15/cm experimentally. Therefore, FIB-DBR or FIB-distributed-feedback (DFB) lasers with performance comparable to that of conventional DBR (or DFB) lasers can be expected.

  19. Optical field ionization of atoms and ions using ultrashort laser pulses

    SciTech Connect

    Fittinghoff, D.N.

    1993-12-01

    This dissertation research is an investigation of the strong optical field ionization of atoms and ions by 120-fs, 614-run laser pulses and 130-fs, 800-nm laser pulses. The experiments have shown ionization that is enhanced above the predictions of sequential tunneling models for He{sup +2}, Ne{sup +2} and Ar{sup +2}. The ion yields for He{sup +l}, Ne{sup +l} and Ar{sup +l} agree well with the theoretical predictions of optical tunneling models. Investigation of the polarization dependence of the ionization indicates that the enhancements are consistent with a nonsequential ionization mechanism in which the linearly polarized field drives the electron wavefunction back toward the ion core and causes double ionization through inelastic e-2e scattering. These investigations have initiated a number of other studies by other groups and are of current scientific interest in the fields of high-irradiance laser-matter interactions and production of high-density plasmas. This work involved: (1) Understanding the characteristic nature of the ion yields produced by tunneling ionization through investigation of analytic solutions for tunneling at optical frequencies. (2) Extensive characterization of the pulses produced by 614-nm and 800-ran ultrashort pulse lasers. Absolute calibration of the irradiance scale produced shows the practicality of the inverse problem--measuring peak laser irradiance using ion yields. (3) Measuring the ion yields for three noble gases using linear, circular and elliptical polarizations of laser pulses at 614-nm and 800-nm. The measurements are some of the first measurements for pulse widths as low as 120-fs.

  20. Modelling of radiation losses for ion acceleration at ultra-high laser intensities

    NASA Astrophysics Data System (ADS)

    Capdessus, Remi; d'Humières, Emmanuel; Tikhonchuk, Vladimir

    2013-11-01

    Radiation losses of charged particles can become important in ultra high intensity laser plasma interaction. This process is described by the radiation back reaction term in the electron equation of motion. This term is implemented in the relativistic particle-in-cell code by using a renormalized Lorentz-Abraham-Dirac model. In the hole boring regime case of laser ion acceleration it is shown that radiation losses results in a decrease of the piston velocity.

  1. Step density model of laser sustained ion channel and Coulomb explosion

    SciTech Connect

    Rajouria, Satish Kumar; Malik, H. K.; Tripathi, V. K.; Kumar, Pawan

    2015-02-15

    An analytical model of laser sustained ion channel in plasma is developed, assuming electron density to be zero in the inner region and constant outside. The radius of the channel is such that the ponderomotive force on electrons at the channel boundary is balanced by the channel space charge force. The laser is TM eigen mode of the system with Bessel function profile in the interior and modified Bessel function outside. The channel radius increases with laser intensity and the ratio of laser frequency to plasma frequency. Ion Coulomb explosion of the channel, on longer time scale, produces ion energy distribution, an increasing function of energy with a sharp cutoff equal to electron ponderomotive energy at the channel boundary. At peak laser intensity ≈2×10{sup 19}W/cm{sup 2} at 1 μm wavelength and spot size of 8 μm, the cutoff ion energy in a plasma of density ∼10{sup 19}cm{sup −3} is ∼0.73 MeV.

  2. Proof-of-concept experiment for on-line laser induced breakdown spectroscopy analysis of impurity layer deposited on optical window and other plasma facing components of Aditya tokamak

    SciTech Connect

    Maurya, Gulab Singh; Kumar, Rohit; Rai, Awadhesh Kumar; Kumar, Ajai

    2015-12-15

    In the present manuscript, we demonstrate the design of an experimental setup for on-line laser induced breakdown spectroscopy (LIBS) analysis of impurity layers deposited on specimens of interest for fusion technology, namely, plasma-facing components (PFCs) of a tokamak. For investigation of impurities deposited on PFCs, LIBS spectra of a tokamak wall material like a stainless steel sample (SS304) have been recorded through contaminated and cleaned optical windows. To address the problem of identification of dust and gases present inside the tokamak, we have shown the capability of the apparatus to record LIBS spectra of gases. A new approach known as “back collection method” to record LIBS spectra of impurities deposited on the inner surface of optical window is presented.

  3. Proof-of-concept experiment for on-line laser induced breakdown spectroscopy analysis of impurity layer deposited on optical window and other plasma facing components of Aditya tokamak

    NASA Astrophysics Data System (ADS)

    Maurya, Gulab Singh; Kumar, Rohit; Kumar, Ajai; Rai, Awadhesh Kumar

    2015-12-01

    In the present manuscript, we demonstrate the design of an experimental setup for on-line laser induced breakdown spectroscopy (LIBS) analysis of impurity layers deposited on specimens of interest for fusion technology, namely, plasma-facing components (PFCs) of a tokamak. For investigation of impurities deposited on PFCs, LIBS spectra of a tokamak wall material like a stainless steel sample (SS304) have been recorded through contaminated and cleaned optical windows. To address the problem of identification of dust and gases present inside the tokamak, we have shown the capability of the apparatus to record LIBS spectra of gases. A new approach known as "back collection method" to record LIBS spectra of impurities deposited on the inner surface of optical window is presented.

  4. Proof-of-concept experiment for on-line laser induced breakdown spectroscopy analysis of impurity layer deposited on optical window and other plasma facing components of Aditya tokamak.

    PubMed

    Maurya, Gulab Singh; Kumar, Rohit; Kumar, Ajai; Rai, Awadhesh Kumar

    2015-12-01

    In the present manuscript, we demonstrate the design of an experimental setup for on-line laser induced breakdown spectroscopy (LIBS) analysis of impurity layers deposited on specimens of interest for fusion technology, namely, plasma-facing components (PFCs) of a tokamak. For investigation of impurities deposited on PFCs, LIBS spectra of a tokamak wall material like a stainless steel sample (SS304) have been recorded through contaminated and cleaned optical windows. To address the problem of identification of dust and gases present inside the tokamak, we have shown the capability of the apparatus to record LIBS spectra of gases. A new approach known as "back collection method" to record LIBS spectra of impurities deposited on the inner surface of optical window is presented.

  5. Ion and electron emission from silver nanoparticles in intense laser fields

    SciTech Connect

    Doeppner, T.; Fennel, Th.; Radcliffe, P.; Tiggesbaeumker, J.; Meiwes-Broer, K.-H.

    2006-03-15

    By a comparative analysis of the emission of highly charged ions and energetic electrons the interaction dynamics of intense femtosecond laser fields (10{sup 13}-10{sup 14} W/cm{sup 2}) with nanometer-sized silver clusters is investigated. Using dual laser pulses with variable optical delay the time-dependent cluster response is resolved. A dramatic increase both in the atomic charge state of the ions and the maximum electron kinetic energy is observed for a certain delay of the pulses. Corresponding Vlasov calculations on a metal cluster model system indicate that enhanced cluster ionization as well as the generation of fast electrons coincide with resonant plasmon excitation.

  6. Fast ion emission and parametric instabilities in laser-solid target interaction

    NASA Astrophysics Data System (ADS)

    Curcio, A.; Andreoli, P.; Barbarino, M.; Bonasera, A.; Cipriani, M.; Consoli, F.; Cristofari, G.; De Angelis, R.; Di Giorgio, G.; Galletti, M.; Giulietti, D.; Ingenito, F.

    2016-04-01

    The spectrum of the accelerated ions at the laser ABC of ENEA research institute, detected by time of flight measurements, is correlated to the onset of parametric instabilities, evidenced by optical diagnostics. In fact, the emission of the laser harmonics, 2ω and 3/2ω, in the visible spectrum manifests the existence, inside the inhomogeneous plasma, of regions in which electron plasma waves can be generated. These waves are the tool for the production of a supra-thermal electron population, responsible for the creation of an electric potential at the plasma sheath, which drives the ion acceleration.

  7. Swift and heavy ion implanted chalcogenide laser glass waveguides and their different refractive index distributions

    SciTech Connect

    Qiu Feng; Narusawa, Tadashi; Zheng Jie

    2011-02-10

    Planar waveguides have been fabricated in Nd- or Ho-doped gallium lanthanum sulfide laser glasses by 60 MeV Ar or 20 MeV N ion implantation. The refractive index profiles were reconstructed based on the results of prism coupling. The Ar implanted waveguides exhibit an approximate steplike distribution, while the N implanted ones show a ''well + barrier'' type. This difference can be attributed to the much lower dose of Ar ions. After annealing, the N implanted waveguides can support two modes at 1539 nm and have low propagation loss, which makes them candidates for novel waveguide lasers.

  8. Investigation of ion acceleration mechanism through laser-matter interaction in femtosecond domain

    NASA Astrophysics Data System (ADS)

    Altana, C.; Muoio, A.; Lanzalone, G.; Tudisco, S.; Brandi, F.; Cirrone, G. A. P.; Cristoforetti, G.; Fazzi, A.; Ferrara, P.; Fulgentini, L.; Giove, D.; Koester, P.; Labate, L.; Mascali, D.; Palla, D.; Schillaci, F.; Gizzi, L. A.

    2016-09-01

    An experimental campaign aiming to investigate the ion acceleration mechanisms through laser-matter interaction in the femtosecond domain has been carried out at the ILIL facility at a laser intensity of up to 2×1019 W/cm2. A Thomson Parabola Spectrometer was used to identify different ion species and measure the energy spectra and the corresponding temperature parameters. We discuss the dependence of the protons spectra upon the structural characteristics of the targets (thickness and atomic mass) and the role of surface versus target bulk during acceleration process.

  9. Ablation plasma transport using multicusp magnetic field for laser ion source

    NASA Astrophysics Data System (ADS)

    Takahashi, K.; Umezawa, M.; Uchino, T.; Ikegami, K.; Sasaki, T.; Kikuchi, T.; Harada, N.

    2016-05-01

    We propose a plasma guiding method using multicusp magnetic field to transport the ablation plasma keeping the density for developing laser ion sources. To investigate the effect of guiding using the magnetic field on the ablation plasma, we demonstrated the transport of the laser ablation plasma in the multicusp magnetic field. The magnetic field was formed with eight permanent magnets and arranged to limit the plasma expansion in the radial direction. We investigated the variation of the plasma ion current density and charge distribution during transport in the magnetic field. The results indicate that the plasma is confined in the radial direction during the transport in the multicusp magnetic field.

  10. Method of making an ion-implanted planar-buried-heterostructure diode laser

    DOEpatents

    Brennan, Thomas M.; Hammons, Burrell E.; Myers, David R.; Vawter, Gregory A.

    1992-01-01

    Planar-buried-heterostructure, graded-index, separate-confinement-heterostructure semiconductor diode laser 10 includes a single quantum well or multi-quantum well active stripe 12 disposed between a p-type compositionally graded Group III-V cladding lever 14 and an n-type compositionally graded Group III-V cladding layer 16. The laser 10 includes an iion implanted n-type region 28 within the p-type cladding layer 14 and further includes an ion implanted p-type region 26 within the n-type cladding layer 16. The ion implanted regions are disposed for defining a lateral extent of the active stripe.

  11. Expansion Discharge Source for Ion Beam Laser Spectroscopy of Cold Molecular Ions

    NASA Astrophysics Data System (ADS)

    Porambo, Michael; Pearson, Jessica; Riccardo, Craig; McCall, Benjamin J.

    2013-06-01

    Molecular ions are important in several fields of research, and spectroscopy acts as a key tool in the study of these ions. However, problems such as low ion abundance, ion-neutral confusion, and spectral congestion due to high internal temperatures can hinder effective spectroscopic studies. To circumvent these problems, we are developing a technique called Sensitive, Cooled, Resolved, Ion BEam Spectroscopy (SCRIBES). This ion beam spectrometer will feature a continuous supersonic expansion discharge source to produce cold molecular ions, electrostatic ion optics to focus the ions into an ion beam and bend the beam away from co-produced neutral molecules, an overlap region for cavity enhanced spectroscopy, and a time-of-flight mass spectrometer. When completed, SCRIBES will be an effective tool for the study of large, fluxional, and complex molecular ions that are difficult to study with other means. The ion beam spectrometer has been successfully implemented with a hot ion source. This talk will focus on the work of integrating a supersonic expansion discharge source into the instrument. To better understand how the source would work in the whole ion beam instrument, characterization studies are being performed with spectroscopy of HN_2^+ in a section of the system to ascertain the rotational temperature of the ion expansion. Attempts are also underway to measure the ion current from a beam formed from the expansion. Once the source in this environment is properly understood, we will reintegrate it to the rest of the ion beam system, completing SCRIBES. A. A. Mills, B. M. Siller, M. W. Porambo, M. Perera, H. Kreckel and B. J. McCall J. Chem. Phys., 135, 224201, (2011). K. N. Crabtree, C. A. Kauffman and B. J. McCall Rev. Sci. Instrum. 81, 086103, (2010).

  12. Surface, electrical and mechanical modifications of PMMA after implantation with laser produced iron plasma ions

    NASA Astrophysics Data System (ADS)

    Ahmed, Qazi Salman; Bashir, Shazia; Jalil, Sohail Abdul; Shabbir, Muhammad Kaif; Mahmood, Khaliq; Akram, Mahreen; Khalid, Ayesha; Yaseen, Nazish; Arshad, Atiqa

    2016-07-01

    Laser Produced Plasma (LPP) was employed as an ion source for the modifications in surface, electrical and mechanical properties of poly methyl (methacrylate) PMMA. For this purpose Nd:YAG laser (532 nm, 6 ns, 10 Hz) at a fluence of 12.7 J/cm2 was employed to generate Fe plasma. The fluence and energy measurements of laser produced Fe plasma ions were carried out by employing Thomson Parabola Technique in the presence of magnetic field strength of 0.5 T, using CR-39 as Solid State Nuclear Track Detector (SSNTD). It has been observed that ion fluence ejecting from ablated plasma was maximum at an angle of 5° with respect to the normal to the Fe target surface. PMMA substrates were irradiated with Fe ions of constant energy of 0.85 MeV at various ion fluences ranging from 3.8 × 106 ions/cm2 to 1.8 × 108 ions/cm2 controlled by varying laser pulses from 3000 to 7000. Optical microscope and Scanning Electron Microscope (SEM) were utilized for the analysis of surface features of irradiated PMMA. Results depicted the formation of chain scission, crosslinking, dendrites and star like structures. To explore the electrical behavior, four probe method was employed. The electrical conductivity of ion irradiated PMMA was increased with increasing ion fluence. The surface hardness was measured by shore D hardness tester and results showed the monotonous increment in surface hardness with increasing ion fluence. The increasing trend of surface hardness and electrical conductivity with increasing Fe ion fluence has been well correlated with the surface morphology of ion implanted PMMA. The temperature rise of PMMA surface due to Fe ion irradiation is evaluated analytically and comes out to be in the range of 1.72 × 104 to 1.82 × 104 K. The values of total Linear Energy Transfer (LET) or stopping power of 0.8 MeV Fe ions in PMMA is 61.8 eV/Å and their range is 1.34 μm evaluated by SRIM simulation.

  13. Investigation of effect of solenoid magnet on emittances of ion beam from laser ablation plasma

    SciTech Connect

    Ikeda, Shunsuke Sekine, Megumi; Romanelli, Mark; Cinquegrani, David; Kumaki, Masafumi; Fuwa, Yasuhiro; Kanesue, Takeshi; Okamura, Masahiro; Horioka, Kazuhiko

    2014-02-15

    A magnetic field can increase an ion current of a laser ablation plasma and is expected to control the change of the plasma ion current. However, the magnetic field can also make some fluctuations of the plasma and the effect on the beam emittance and the emission surface is not clear. To investigate the effect of a magnetic field, we extracted the ion beams under three conditions where without magnetic field, with magnetic field, and without magnetic field with higher laser energy to measure the beam distribution in phase space. Then we compared the relations between the plasma ion current density into the extraction gap and the Twiss parameters with each condition. We observed the effect of the magnetic field on the emission surface.

  14. Investigation of effect of solenoid magnet on emittances of ion beam from laser ablation plasma.

    PubMed

    Ikeda, Shunsuke; Romanelli, Mark; Cinquegrani, David; Sekine, Megumi; Kumaki, Masafumi; Fuwa, Yasuhiro; Kanesue, Takeshi; Okamura, Masahiro; Horioka, Kazuhiko

    2014-02-01

    A magnetic field can increase an ion current of a laser ablation plasma and is expected to control the change of the plasma ion current. However, the magnetic field can also make some fluctuations of the plasma and the effect on the beam emittance and the emission surface is not clear. To investigate the effect of a magnetic field, we extracted the ion beams under three conditions where without magnetic field, with magnetic field, and without magnetic field with higher laser energy to measure the beam distribution in phase space. Then we compared the relations between the plasma ion current density into the extraction gap and the Twiss parameters with each condition. We observed the effect of the magnetic field on the emission surface.

  15. Generation of circularly polarized attosecond pulses by intense ultrashort laser pulses from extended asymmetric molecular ions

    SciTech Connect

    Yuan, Kai-Jun; Bandrauk, Andre D.

    2011-08-15

    We present a method for generation of single circularly polarized attosecond pulses in extended asymmetric HHe{sup 2+} molecular ions. By employing an intense ultrashort circularly polarized laser pulse with intensity 4.0x10{sup 14} W/cm{sup 2}, wavelength 400 nm, and duration 10 optical cycles, molecular high-order-harmonic generation (MHOHG) spectra with multiple plateaus exhibit characters of circular polarization. Using a classical laser-induced collision model, double collisions of continuum electrons first with neighboring ions and then second with parent ions are presented at a particular internuclear distance and confirmed from numerical solutions of a time-dependent Schroedinger equation. We analyze the MHOHG spectra with a Gabor time window and find that, due to the asymmetry of HHe{sup 2+}, a single collision trajectory of continuum electrons with ions can produce circularly polarized harmonics, leading to single circularly polarized attosecond pulses for specific internuclear distances.

  16. Ultraintense laser interaction with nanoscale target: a simple model for layer expansion and ion acceleration

    SciTech Connect

    Albright, Brian J; Yin, Lin; Hegelich, Bjoorn M; Bowers, Kevin J; Huang, Chengkun; Fernandez, Juan C; Flippo, Kirk A; Gaillard, Sandrine; Kwan, Thomas J T; Henig, Andreas; Yan, Xue Q; Tajima, Toshi; Habs, Dieter

    2009-01-01

    A simple model has been derived for the expansion of a thin (up to 100s of nm thickness), solid-density target driven by an u.ltraintense laser. In this regime, new ion acceleration mechanisms, such as the Break-Out Afterburner (BOA) [1], emerge with the potential to dramatically improve energy, efficiency, and energy spread of laser-driven ion beams. Such beams have been proposed [2] as drivers for fast ignition inertial confinement fusion [3]. Analysis of kinetic simulations of the BOA shows two dislinct times that bound the period of enhanced acceleration: t{sub 1}, when the target becomes relativistically transparent to the laser, and t{sub 2}, when the target becomes classically underdense and the enhanced acceleration terminates. A silllple dynamical model for target expansion has been derived that contains both the early, one-dimensional (lD) expansion of the target as well as three-dimensional (3D) expansion of the plasma at late times, The model assumes that expansion is slab-like at the instantaneous ion sound speed and requires as input target composition, laser intensity, laser spot area, and the efficiency of laser absorption into electron thermal energy.

  17. Key conditions for stable ion radiation pressure acceleration by circularly polarized laser pulses

    NASA Astrophysics Data System (ADS)

    Qiao, B.; Zepf, M.; Gibbon, P.; Borghesi, M.; Schreiber, J.; Geissler, M.

    2011-05-01

    Radiation pressure acceleration (RPA) theoretically may have great potential to revolutionize the study of laserdriven ion accelerators due to its high conversion efficiency and ability to produce high-quality monoenergetic ion beams. However, the instability issue of ion acceleration has been appeared to be a fundamental limitation of the RPA scheme. To solve this issue is very important to the experimental realization and exploitation of this new scheme. In our recent work, we have identified the key condition for efficient and stable ion RPA from thin foils by CP laser pulses, in particular, at currently available moderate laser intensities. That is, the ion beam should remain accompanied with enough co-moving electrons to preserve a local "bunching" electrostatic field during the acceleration. In the realistic LS RPA, the decompression of the co-moving electron layer leads to a change of local electrostatic field from a "bunching" to a "debunching" profile, resulting in premature termination of acceleration. One possible scheme to achieve stable RPA is using a multi-species foil. Two-dimensional PIC simulations show that 100 MeV/u monoenergetic C6+ and/or proton beams are produced by irradiation of a contaminated copper foil with CP lasers at intensities 5 × 1020W/cm2, achievable by current day lasers.

  18. Numerical study of neutron beam divergence in a beam-fusion scenario employing laser driven ions

    NASA Astrophysics Data System (ADS)

    Alejo, A.; Green, A.; Ahmed, H.; Robinson, A. P. L.; Cerchez, M.; Clarke, R.; Doria, D.; Dorkings, S.; Fernandez, J.; McKenna, P.; Mirfayzi, S. R.; Naughton, K.; Neely, D.; Norreys, P.; Peth, C.; Powell, H.; Ruiz, J. A.; Swain, J.; Willi, O.; Borghesi, M.; Kar, S.

    2016-09-01

    The most established route to create a laser-based neutron source is by employing laser accelerated, low atomic-number ions in fusion reactions. In addition to the high reaction cross-sections at moderate energies of the projectile ions, the anisotropy in neutron emission is another important feature of beam-fusion reactions. Using a simple numerical model based on neutron generation in a pitcher-catcher scenario, anisotropy in neutron emission was studied for the deuterium-deuterium fusion reaction. Simulation results are consistent with the narrow-divergence (∼ 70 ° full width at half maximum) neutron beam recently served in an experiment employing multi-MeV deuteron beams of narrow divergence (up to 30° FWHM, depending on the ion energy) accelerated by a sub-petawatt laser pulse from thin deuterated plastic foils via the Target Normal Sheath Acceleration mechanism. By varying the input ion beam parameters, simulations show that a further improvement in the neutron beam directionality (i.e. reduction in the beam divergence) can be obtained by increasing the projectile ion beam temperature and cut-off energy, as expected from interactions employing higher power lasers at upcoming facilities.

  19. Threshold level laser photoablation of crystalline silver: Ejected ion translational energy distributions

    NASA Astrophysics Data System (ADS)

    Helvajian, H.; Welle, R.

    1989-08-01

    We have conducted an experiment which measures, for a single laser shot, the ejected mass and nascent velocity distributions of ionic species ablated at laser fluences near the threshold for ion production. Our results show that for a crystalline silver target, the laser-ablated ion products are ejected with fixed kinetic energy equal to 9±1 eV (3 eV FWHM). The kinetic energy of the ejecta (Ag+,Ag+2, adsorbed Fe+) do not vary with wavelength (351 and 248 nm), nor with the ion product mass, and within limits are independent of the incident laser intensity. We do see a wavelength dependence in the threshold for ion production and in the dimer/monomer (Ag+/Ag+2) ion ratio. A number of possible mechanisms are presented to explain the data, although none is without some objection. Among these, the process whereby desorption is induced by electronic transitions (DIET processes) has some merit in explaining our data.

  20. Multidiagnostic analysis of ion dynamics in ultrafast laser ablation of metals over a large fluence range

    SciTech Connect

    Anoop, K. K. Bruzzese, R.; Amoruso, S.; Polek, M. P.; Harilal, S. S.

    2015-02-28

    The dynamics of ions in ultrafast laser ablation of metals is studied over fluences ranging from the ablation threshold up to ≈75 J/cm{sup 2} by means of three well-established diagnostic techniques. Langmuir probe, Faraday cup, and spectrally resolved intensified charge coupled device imaging simultaneously monitored the ions produced during ultrafast laser ablation of a pure copper target with 800 nm, ≈50 fs, Ti: Sapphire laser pulses. The fluence dependence of ion yield is analyzed, resulting in the observance of three different regimes. The specific ion yield shows a maximum at about 4–5 J/cm{sup 2}, followed by a gradual reduction and a transition to a high-fluence regime above ≈50 J/cm{sup 2}. The fluence dependence of the copper ions angular distribution is also analyzed, observing a gradual increase in forward-peaking of Cu ions for fluences up to ≈10 J/cm{sup 2}. A broader ion component is observed at larger angles for fluences larger than ≈10 J/cm{sup 2}. Finally, an experimental characterization of the ionic angular distribution for several metallic targets (Mg, Al, Cr, Fe, Cu, and W) is carried out at a relatively high fluence of ≈66 J/cm{sup 2}. Interestingly, the ion emission from the volatile metals shows a narrow, forward-peaked distribution, and a high peak ion yield compared to the refractory metals. Moreover, the width of ionic angular distributions presents a striking correlation with the peak ion yield.

  1. Performance on the low charge state laser ion source in BNL

    SciTech Connect

    Okamura, M.; Alessi, J.; Beebe, E.; Costanzo, M.; DeSanto, L.; Jamilkowski, J.; Kanesue, T.; Lambiase, R.; Lehn, D.; Liaw, C. J.; McCafferty, D.; Morris, J.; Olsen, R.; Pikin, A.; Raparia, D.; Steszyn, A.; Ikeda, S.

    2015-09-07

    On March 2014, a Laser Ion Source (LIS) was commissioned which delivers high-brightness, low-charge-state heavy ions for the hadron accelerator complex in Brookhaven National Laboratory (BNL). Since then, the LIS has provided many heavy ion species successfully. The low-charge-state (mostly singly charged) beams are injected to the Electron Beam Ion Source (EBIS), where ions are then highly ionized to fit to the following accelerator’s Q/M acceptance, like Au32+. Recently we upgraded the LIS to be able to provide two different beams into EBIS on a pulse-to-pulse basis. Now the LIS is simultaneously providing beams for both the Relativistic Heavy Ion Collider (RHIC) and NASA Space Radiation Laboratory (NSRL).

  2. A carbon-cluster laser ion source for TRIGA-TRAP

    NASA Astrophysics Data System (ADS)

    Smorra, C.; Blaum, K.; Eberhardt, K.; Eibach, M.; Ketelaer, J.; Ketter, J.; Knuth, K.; Nagy, Sz

    2009-08-01

    A new laser ablation ion source was developed and tested for the Penning trap mass spectrometer TRIGA-TRAP in order to provide carbon-cluster ions for absolute mass calibration. Ions of different cluster sizes up to C+24 were successfully produced, covering the mass range up to the heavy actinide elements. The ions were captured in a Penning trap, and their time-of-flight cyclotron resonances recorded in order to determine their cyclotron frequency. Furthermore, the same ion source was used to produce GdO+ ions from a gadolinium target in sufficient amount for mass spectrometry purposes. The design of the source and its characteristics are presented. This paper comprises partly the PhD theses of J Ketelaer and C Smorra.

  3. Laser-induced fluorescence and nonlinear optical properties of ion-implanted fused silica

    SciTech Connect

    Becker, K.; Yang, L.; Haglund, R.F. Jr. . Dept. of Physics and Astronomy); Magruder, R.H.; Weeks, R.A. . Dept. of Materials Science and Engineering); Zuhr, R.A. )

    1990-01-01

    We report absorption, fluorescence and nonlinear optical properties of fused silica implanted with Ti, Cu and Bi and doses of 1{center dot}10{sup 15} ions/cm{sup 2} to 6{center dot}10{sup 16} ions/cm{sup 2} when irradiated with 532 nm laser light. The fluorescence spectrum is a broad band around 640 nm shows little variation for all ion species. Absorption as function of implanted dose shows a threshold for Ti between 1{center dot}10{sup 16} ions/cm{sup 2} and 6{center dot}10{sup 16} ions/cm{sup 2}. The nonlinear optical index is large, n{sub 2} > 10{sup {minus}5} esu. All measured quantities show a strong dependence on the implanted ion dose. The source of the nonlinearity, whether electronic or thermal, remains to be more completely determined. 9 refs., 4 figs.

  4. Development of Laser-Ion Beam Photodissociation Methods

    SciTech Connect

    David H. Russell

    2004-05-11

    OAK-B135 Our BES funded research is aimed at determining structure(s) of model gas-phase ions and understanding how structure influences unimolecular reactivity. The model gas-phase ions include positional isomers of di- and tri-amino acids synthesized in my laboratory, i.e., RGG, GRG, and GGR, to peptides derived from proteolytic digestion of biologically relevant proteins. We are especially interested in understanding the role of intramolecular interactions in the stabilizing ion structure and how changing the charge-site affects structure. The location of charge of gas-phase ions can be manipulated by changing the position of the charge carrying amino acid (basic vs. acidic side chains) and by derivatization of the N- and/or C-terminus. For example, the proton of [M + H]+ ions is mobile and migrates over the entire molecule, whereas Li+, Na+, and to some extent K+ prefers to bind to the C-terminal or side-chain carboxylic acid groups, and Cu+ binds exclusively to the N-terminus and/or basic side-chains such as H, K, and R. The studies are carried out using tandem TOF mass spectrometry, viz. 193 nm (6.43 eV) photodissociation, low (Elab = 10-100 eV) and high kinetic energy (Elab = 1-10 keV) collision-induced dissociation (CID) and surface-induced dissociation (SID)(Elab = 20-70 eV). These techniques are used to probe the structure of model gas-phase ions, i.e., to determine the amino acid sequence of the peptide ions or metal ion (alkali metal and/or transition metal ions) binding site(s) or the site(s) of other charge-carrying functional groups, i.e., oxidized side-chains as well as phosphate or sulfate groups. We are especially interested in understanding how metal ion binding alters the secondary/tertiary (2o/3o) structure of the peptide, i.e., intra-molecular interactions. We have also combine these studies with solution-phase studies and ion mobility spectrometry (IMS)), which can be used to study 2o/3o structure of low-internal energy (collisionally

  5. Development of Laser-Ion Beam Photodissociation Methods

    SciTech Connect

    David H. Russell

    2004-03-31

    OAK-B135 Our BES funded research is aimed at determining structure(s) of model gas-phase ions and understanding how structure influences unimolecular reactivity. The model gas-phase ions include positional isomers of di- and tri-amino acids synthesized in my laboratory, i.e., RGG, GRG, and GGR, to peptides derived from proteolytic digestion of biologically relevant proteins. We are especially interested in understanding the role of intramolecular interactions in the stabilizing ion structure and how changing the charge-site affects structure. The location of charge of gas-phase ions can be manipulated by changing the position of the charge carrying amino acid (basic vs. acidic side chains) and by derivatization of the N- and/or C-terminus. For example, the proton of [M + H]+ ions is mobile and migrates over the entire molecule, whereas Li+, Na+, and to some extent K+ prefers to bind to the C-terminal or side-chain carboxylic acid groups, and Cu+ binds exclusively to the N-terminus and/or basic side-chains such as H, K, and R. The studies are carried out using tandem TOF mass spectrometry, viz. 193 nm (6.43 eV) photodissociation, low (Elab = 10-100 eV) and high kinetic energy (Elab = 1-10 keV) collision-induced dissociation (CID) and surface-induced dissociation (SID)(Elab = 20-70 eV). These techniques are used to probe the structure of model gas-phase ions, i.e., to determine the amino acid sequence of the peptide ions or metal ion (alkali metal and/or transition metal ions) binding site(s) or the site(s) of other charge-carrying functional groups, i.e., oxidized side-chains as well as phosphate or sulfate groups. We are especially interested in understanding how metal ion binding alters the secondary/tertiary (2o/3o) structure of the peptide, i.e., intra-molecular interactions. We have also combine these studies with solution-phase studies and ion mobility spectrometry (IMS), which can be used to study 2o/3o structure of low-internal energy (collisionally

  6. Experimental study of the ion emission from a 0. 53-. mu. m laser-produced plasma

    SciTech Connect

    Kieffer, J.C.; Quemener, Y.; Briand, J.; Gomes, A.; Adrian, V.; Dinguirard, J.P.; Armengaud, M.; Thoron, J.P.; Fournier, N.; El Tamer, M.

    1985-12-15

    Ion velocity distributions generated in a 0.53-..mu..m laser-produced plasma are studied with a Thomson parabola diagnostic at 5 x 10/sup 13/ W/cm/sup 2/. Ions are observed in a narrow energy range. However, for velocities >4 x 10/sup 5/ m/s the distribution dN/dV decreases exponentially and the temperatures deduced from these distributions are in good agreement with those given by x-ray emission.

  7. Static testing system for optical disks with an argon ion laser

    NASA Astrophysics Data System (ADS)

    Zhang, Guoxuan; Xu, Wendong; Ge, Hezong; Men, Liqiu Q.; Gan, Baihui; Yu, Dunhe

    1996-09-01

    We have developed a testing system with 514.5 nm argon ion laser to test the static properties of optical disks. The whole testing system is controlled by a computer. The laser power, pulse duration time and external applied magnetic field can be adjusted in a wide range. The focused spot size is less than 1 micrometers on the recording layer which allows high laser power irradiation, up to 30 mW. This testing system can evaluate the writing and erasing characteristics of phase-changes and magneto-optical disks. The design idea and experimental results of this testing system are presented.

  8. Hybrid ion acceleration with ultrathin composite foils irradiated by high intensity circularly-polarized laser light

    SciTech Connect

    Andreev, A. A.; Steinke, S.; Schnuerer, M.; Sokollik, T.; Sandner, W.; Henig, A.; Nickles, P. V.; Platonov, K. Y.

    2010-12-15

    A complete analytical description of ion acceleration in the laser radiation-pressure regime is presented. The combined effects of hot electron and light-pressure phenomena are used to qualitatively and quantitatively describe most recent experimental results in this regime. An essential part of the developed model is exhibited in the calculation of nonlinear laser light reflection and transmission properties, as well as in the spectral characterization of the laser light after interaction. The validity of the analytical model is supported by recent experimental results and by particle-in-cell simulations.

  9. Laser Ablation Electrodynamic Ion Funnel for In Situ Mass Spectrometry on Mars

    NASA Technical Reports Server (NTRS)

    Johnson, Paul V.; Hodyss, Robert P.; Tang, Keqi; Smith, Richard D.

    2012-01-01

    A front-end instrument, the laser ablation ion funnel, was developed, which would ionize rock and soil samples in the ambient Martian atmosphere, and efficiently transport the product ions into a mass spectrometer for in situ analysis. Laser ablation creates elemental ions from a solid with a high-power pulse within ambient Mars atmospheric conditions. Ions are captured and focused with an ion funnel into a mass spectrometer for analysis. The electrodynamic ion funnel consists of a series of axially concentric ring-shaped electrodes whose inside diameters (IDs) decrease over the length of the funnel. DC potentials are applied to each electrode, producing a smooth potential slope along the axial direction. Two radio-frequency (RF) AC potentials, equal in amplitude and 180 out of phase, are applied alternately to the ring electrodes. This creates an effective potential barrier along the inner surface of the electrode stack. Ions entering the funnel drift axially under the influence of the DC potential while being restricted radially by the effective potential barrier created by the applied RF. The net result is to effectively focus the ions as they traverse the length of the funnel.

  10. Bright focused ion beam sources based on laser-cooled atoms

    PubMed Central

    McClelland, J. J.; Steele, A. V.; Knuffman, B.; Twedt, K. A.; Schwarzkopf, A.; Wilson, T. M.

    2016-01-01

    Nanoscale focused ion beams (FIBs) represent one of the most useful tools in nanotechnology, enabling nanofabrication via milling and gas-assisted deposition, microscopy and microanalysis, and selective, spatially resolved doping of materials. Recently, a new type of FIB source has emerged, which uses ionization of laser cooled neutral atoms to produce the ion beam. The extremely cold temperatures attainable with laser cooling (in the range of 100 μK or below) result in a beam of ions with a very small transverse velocity distribution. This corresponds to a source with extremely high brightness that rivals or may even exceed the brightness of the industry standard Ga+ liquid metal ion source. In this review we discuss the context of ion beam technology in which these new ion sources can play a role, their principles of operation, and some examples of recent demonstrations. The field is relatively new, so only a few applications have been demonstrated, most notably low energy ion microscopy with Li ions. Nevertheless, a number of promising new approaches have been proposed and/or demonstrated, suggesting that a rapid evolution of this type of source is likely in the near future. PMID:27239245

  11. Bright focused ion beam sources based on laser-cooled atoms

    NASA Astrophysics Data System (ADS)

    McClelland, J. J.; Steele, A. V.; Knuffman, B.; Twedt, K. A.; Schwarzkopf, A.; Wilson, T. M.

    2016-03-01

    Nanoscale focused ion beams (FIBs) represent one of the most useful tools in nanotechnology, enabling nanofabrication via milling and gas-assisted deposition, microscopy and microanalysis, and selective, spatially resolved doping of materials. Recently, a new type of FIB source has emerged, which uses ionization of laser cooled neutral atoms to produce the ion beam. The extremely cold temperatures attainable with laser cooling (in the range of 100 μK or below) result in a beam of ions with a very small transverse velocity distribution. This corresponds to a source with extremely high brightness that rivals or may even exceed the brightness of the industry standard Ga+ liquid metal ion source. In this review, we discuss the context of ion beam technology in which these new ion sources can play a role, their principles of operation, and some examples of recent demonstrations. The field is relatively new, so only a few applications have been demonstrated, most notably low energy ion microscopy with Li ions. Nevertheless, a number of promising new approaches have been proposed and/or demonstrated, suggesting that a rapid evolution of this type of source is likely in the near future.

  12. Highly-charged heavy-ion production with short pulse lasers

    SciTech Connect

    Logan, G.; Bitmire, T.; Perry, M.; Anderson, O.; Kuehl, T.

    1998-01-27

    This MathCAD document describes a possible approach using a PW -class short pulse laser to form a useful number (10{sup 12}) of high and uniform charge state ions with low ion temperature (<< 100 eV) and low momentum spread ({delta}p{sub z}/p, < 10{sup -4} ) for injection into heavy-ion fusion accelerators. As a specific example, we consider here Xenon{sup +26}, which has an ionization energy E{sub i} {approximately} 860 eV for the 26th electron, and a significantly higher ionization potential of 1500 eV for the 27th electron because of the M-shell jump. The approach considered here may be used for other ion species as well. The challenge is not simply to produce high charge states with a laser (the ITEP group [Sharkov] have used long pulse CO{sub 2} lasers to create many charge states of chromium up to helium-like Cr{sup +25} by collisional ionization at high Te), nor just to create such high charge states more selectively by field (tunneling) ionization at higher intensities and shorter pulses. Rather, the challenge is to create a selected uniform high charge state, in useful numbers, while keeping the ion temperature and momentum spread small, and avoiding subsequent loss of ion charge state due to recombination and charge-exchange with background gas atoms during extraction into a useful low emittance beam.

  13. Nanoscale helium ion microscopic analysis of collagen fibrillar changes following femtosecond laser dissection of human cornea.

    PubMed

    Riau, Andri K; Poh, Rebekah; Pickard, Daniel S; Park, Chris H J; Chaurasia, Shyam S; Mehta, Jodhbir S

    2014-08-01

    Over the last decade, femtosecond lasers have emerged as an important tool to perform accurate and fine dissections with minimal collateral damage in biological tissue. The most common surgical procedure in medicine utilizing femtosecond laser is LASIK. During the femtosecond laser dissection process, the corneal collagen fibers inevitably undergo biomechanical and thermal changes on a sub-micro- or even a nanoscale level, which can potentially lead to post-surgical complications. In this study, we utilized helium ion microscopy, complemented with transmission electron microscopy to examine the femtosecond laser-induced collagen fibrillar damage in ex vivo human corneas. We found that the biomechanical damage induced by laser etching, generation of tissue bridges, and expansion of cavitation bubble and its subsequent collapse, created distortion to the surrounding collagen lamellae. Femtosecond laser-induced thermal damage was characterized by collapsed collagen lamellae, loss of collagen banding, collagen coiling, and presence of spherical debris. Our findings have shown the ability of helium ion microscopy to provide high resolution images with unprecedented detail of nanoscale fibrillar morphological changes in order to assess a tissue damage, which could not be resolved by conventional scanning electron microscopy previously. This imaging technology has also given us a better understanding of the tissue-laser interactions in a nano-structural manner and their possible effects on post-operative wound recovery. PMID:25016655

  14. Nanoscale helium ion microscopic analysis of collagen fibrillar changes following femtosecond laser dissection of human cornea.

    PubMed

    Riau, Andri K; Poh, Rebekah; Pickard, Daniel S; Park, Chris H J; Chaurasia, Shyam S; Mehta, Jodhbir S

    2014-08-01

    Over the last decade, femtosecond lasers have emerged as an important tool to perform accurate and fine dissections with minimal collateral damage in biological tissue. The most common surgical procedure in medicine utilizing femtosecond laser is LASIK. During the femtosecond laser dissection process, the corneal collagen fibers inevitably undergo biomechanical and thermal changes on a sub-micro- or even a nanoscale level, which can potentially lead to post-surgical complications. In this study, we utilized helium ion microscopy, complemented with transmission electron microscopy to examine the femtosecond laser-induced collagen fibrillar damage in ex vivo human corneas. We found that the biomechanical damage induced by laser etching, generation of tissue bridges, and expansion of cavitation bubble and its subsequent collapse, created distortion to the surrounding collagen lamellae. Femtosecond laser-induced thermal damage was characterized by collapsed collagen lamellae, loss of collagen banding, collagen coiling, and presence of spherical debris. Our findings have shown the ability of helium ion microscopy to provide high resolution images with unprecedented detail of nanoscale fibrillar morphological changes in order to assess a tissue damage, which could not be resolved by conventional scanning electron microscopy previously. This imaging technology has also given us a better understanding of the tissue-laser interactions in a nano-structural manner and their possible effects on post-operative wound recovery.

  15. Fisher information and Shannon entropy for on-line detection of transient signal high-values in laser Doppler flowmetry signals of healthy subjects

    NASA Astrophysics Data System (ADS)

    Humeau, Anne; Trzepizur, Wojciech; Rousseau, David; Chapeau-Blondeau, François; Abraham, Pierre

    2008-09-01

    Laser Doppler flowmetry (LDF) is an easy-to-use method for the assessment of microcirculatory blood flow in tissues. However, LDF recordings very often present TRAnsient Signal High-values (TRASH), generally of a few seconds. These TRASH can come from tissue motions, optical fibre movements, movements of the probe head relative to the tissue, etc. They often lead to difficulties in signal global interpretations. In order to test the possibility of detecting automatically these TRASH for their removal, we process noisy and noiseless LDF signals with two indices from information theory, namely Fisher information and Shannon entropy. For this purpose, LDF signals from 13 healthy subjects are recorded at rest, during vascular occlusion of 3 min, and during post-occlusive hyperaemia. Computation of Fisher information and Shannon entropy values shows that, when calibrated, these two indices can be complementary to detect TRASH and be insensitive to the rapid increases of blood flow induced by post-occlusive hyperaemia. Moreover, the real-time algorithm has the advantage of being easy to implement and does not require any frequency analysis. This study opens new fields of application for Fisher information and Shannon entropy: LDF 'denoising'.

  16. On-line atomic data access

    NASA Astrophysics Data System (ADS)

    Schultz, David R.; Nash, Jeffrey K.

    1996-07-01

    The need for atomic data is one which continues to expand in a wide variety of applications including fusion energy, astrophysics, laser-produced plasma research, and plasma processing. Modern computer database and communications technology enables this data to be placed on-line and obtained by users over the INTERNET. Presented here is a summary of the observations and conclusions regarding such on-line atomic data access derived from a forum held at the Tenth APS Topical Conference on Atomic Processes in Plasmas.

  17. Effect of the laser spot shape on spatial distribution of the ion bunch accelerated in a superstrong field

    SciTech Connect

    Komarov, V M; Charukhchev, A V; Andreev, A A; Platonov, K Yu

    2014-12-31

    We have investigated the effect of the laser spot shape on the spatial distribution of accelerated ions on the front and back sides of a thin target irradiated by a picosecond laser pulse having the intensity of (3 – 4) × 10{sup 18} W cm{sup -2}. Experimental data are compared with numerical calculations. It is shown that the spatial structure of the ion bunch on the front side of the target resembles the laser spot structure rotated by 90°. (interaction of laser radiation with matter. laser plasma)

  18. Ion flux enhancements and oscillations in spatially confined laser produced aluminum plasmas

    SciTech Connect

    Singh, S. C. Fallon, C.; Hayden, P.; Yeates, P.; Costello, J. T.; Mujawar, M.

    2014-09-15

    Ion signals from laser produced plasmas (LPPs) generated inside aluminum rectangular cavities at a fixed depth d = 2 mm and varying width, x = 1.0, 1.6, and 2.75 mm were obtained by spatially varying the position of a negatively biased Langmuir probe. Damped oscillatory features superimposed on Maxwellian distributed ion signals were observed. Depending on the distance of the probe from the target surface, three to twelve fold enhancements in peak ion density were observed via confinement of the LPP, generated within rectangular cavities of varying width which constrained the plasma plume to near one dimensional expansion in the vertical plane. The effects of lateral spatial confinement on the expansion velocity of the LPP plume front, the temperature, density and expansion velocity of ions, enhancement of ion flux, and ion energy distribution were recorded. The periodic behavior of ion signals was analyzed and found to be related to the electron plasma frequency and electron-ion collision frequency. The effects of confinement and enhancement of various ion parameters and expansion velocities of the LPP ion plume are explained on the basis of shock wave theory.

  19. Ion flux enhancements and oscillations in spatially confined laser produced aluminum plasmas

    NASA Astrophysics Data System (ADS)

    Singh, S. C.; Fallon, C.; Hayden, P.; Mujawar, M.; Yeates, P.; Costello, J. T.

    2014-09-01

    Ion signals from laser produced plasmas (LPPs) generated inside aluminum rectangular cavities at a fixed depth d = 2 mm and varying width, x = 1.0, 1.6, and 2.75 mm were obtained by spatially varying the position of a negatively biased Langmuir probe. Damped oscillatory features superimposed on Maxwellian distributed ion signals were observed. Depending on the distance of the probe from the target surface, three to twelve fold enhancements in peak ion density were observed via confinement of the LPP, generated within rectangular cavities of varying width which constrained the plasma plume to near one dimensional expansion in the vertical plane. The effects of lateral spatial confinement on the expansion velocity of the LPP plume front, the temperature, density and expansion velocity of ions, enhancement of ion flux, and ion energy distribution were recorded. The periodic behavior of ion signals was analyzed and found to be related to the electron plasma frequency and electron-ion collision frequency. The effects of confinement and enhancement of various ion parameters and expansion velocities of the LPP ion plume are explained on the basis of shock wave theory.

  20. Nonlinear study of an ion-channel guiding free-electron laser

    SciTech Connect

    Ouyang, Zhengbiao; Zhang, Shi-Chang

    2015-04-15

    A nonlinear model and simulations of the output power of an ion-channel guiding free-electron laser (FEL) are presented in this paper. Results show that the nonlinear output power of an ion-channel guiding FEL is comparable to that of an axial guide magnetic field FEL. Compared to an axial guide magnetic field FEL, an ion-channel guiding FEL substantially weakens the negative effect of the electron-beam energy spread on the output power due to its advantageous focusing mechanism on the electron motion.

  1. Ultrafast electronic motion in hydrogen molecular ions induced by a high power intense laser

    NASA Astrophysics Data System (ADS)

    Mineo, H.; Teranishi, Y.; Chao, S. D.; Lin, S. H.

    2010-10-01

    In this Letter we report a method for controlling electronic localization in a molecular ion, on an attosecond time scale, using a high-intensity laser, based on two different excitation mechanisms. One takes place during ionization, and the other takes place sequentially, following ionization. The electronic excited states of the hydrogen molecular ion are created during ionization by taking the configuration interaction mixing of neutral molecules into account. We detect the ultrafast oscillatory electronic motion between two atoms in a hydrogen molecular ion occurring due to the creation of excited states during the course of ionization.

  2. Charge equilibrium of a laser-generated carbon-ion beam in warm dense matter.

    PubMed

    Gauthier, M; Chen, S N; Levy, A; Audebert, P; Blancard, C; Ceccotti, T; Cerchez, M; Doria, D; Floquet, V; Lamour, E; Peth, C; Romagnani, L; Rozet, J-P; Scheinder, M; Shepherd, R; Toncian, T; Vernhet, D; Willi, O; Borghesi, M; Faussurier, G; Fuchs, J

    2013-03-29

    Using ion carbon beams generated by high intensity short pulse lasers we perform measurements of single shot mean charge equilibration in cold or isochorically heated solid density aluminum matter. We demonstrate that plasma effects in such matter heated up to 1 eV do not significantly impact the equilibration of carbon ions with energies 0.045-0.5  MeV/nucleon. Furthermore, these measurements allow for a first evaluation of semiempirical formulas or ab initio models that are being used to predict the mean of the equilibrium charge state distribution for light ions passing through warm dense matter. PMID:23581330

  3. Improving beam spectral and spatial quality by double-foil target in laser ion acceleration for ion-driven fast ignition

    SciTech Connect

    Huang, Chengkun; Albright, Brian J

    2010-07-16

    Mid-Z ion driven fast ignition inertial fusion requires ion beams of 100s of MeV energy and < 10% energy spread. An overdense run-scale foil target driven by a high intensity laser pulse can produce an ion beam that has attractive properties for this application. The Break Out Afterburner (BOA) is one laser-ion acceleration mechanism proposed to generate such beams, however the late stages of the BOA tend to produce too large of an energy spread. The spectral and spatial qualities of the beam quickly evolve as the ion beam and co-moving electrons continue to interact with the laser. Here we show how use of a second target foil placed behind a nm-scale foil can substantially reduce the temperature of the co-moving electrons and improve the ion beam energy spread. Particle-In-Cell simulations reveal the dynamics of the ion beam under control. Optimal conditions for improving the spectral and spatial spread of the ion beam is explored for current laser and target parameters, leading to generation of ion beams of energy 100s of MeV and 6% energy spread, a vital step for realizing ion-driven fast ignition.

  4. BRIEF COMMUNICATIONS: Coherent anti-Stokes Raman scattering by excited ions in a laser plasma

    NASA Astrophysics Data System (ADS)

    Gladkov, S. M.; Zheltikov, Aleksei M.; Koroteev, Nikolai I.; Rychev, M. V.; Fedotov, Andrei B.

    1989-07-01

    The coherent anti-Stokes Raman scattering (CARS) method was used in observation of excited Al II, Al III, In II and N II in an optical breakdown plasma. The feasibility of CARS spectroscopy of multiply charged ions in a laser plasma was established.

  5. Controlled Ion Acceleration in Two Crossed Laser Beams Propagating in Plasmas

    NASA Astrophysics Data System (ADS)

    Tataronis, J. A.; Petržílka, V.; Krlín, L.

    2003-10-01

    Electron acceleration occurs in a single plane laser beam that is in the presence of a secondary perpendicularly propagating plane laser beam with a randomized phase. As the accelerated electrons are pushed away, they leave the heavier ions behind, producing thereby a charge separation electrostatic field and consequent ion flows. The power flux carried by the accelerated ions can be controlled by varying the intensity of the secondary beam. Results of a numerical study of this control process are presented here. The laser beam parameters chosen for the computations of the primary electron acceleration match the parameters available at the Prague Asterix Laser System (PALS)^1. For the modeling, we use an advanced version of our 3-d two-fluid numerical code^2, originally developed for the analysis of fast electron generation and subsequent ion acceleration in front of lower hybrid wave launchers in large tokamaks. [2pt] ^1K. Jungwirth et al., Phys. Plasmas 8, 2495 (2001). [2pt] ^2V. Petržílka et al., Proc. 29th EPS Conference, Montreux, June 2002, paper 2.105.

  6. Guided post-acceleration of laser-driven ions by a miniature modular structure

    PubMed Central

    Kar, Satyabrata; Ahmed, Hamad; Prasad, Rajendra; Cerchez, Mirela; Brauckmann, Stephanie; Aurand, Bastian; Cantono, Giada; Hadjisolomou, Prokopis; Lewis, Ciaran L. S.; Macchi, Andrea; Nersisyan, Gagik; Robinson, Alexander P. L.; Schroer, Anna M.; Swantusch, Marco; Zepf, Matt; Willi, Oswald; Borghesi, Marco

    2016-01-01

    All-optical approaches to particle acceleration are currently attracting a significant research effort internationally. Although characterized by exceptional transverse and longitudinal emittance, laser-driven ion beams currently have limitations in terms of peak ion energy, bandwidth of the energy spectrum and beam divergence. Here we introduce the concept of a versatile, miniature linear accelerating module, which, by employing laser-excited electromagnetic pulses directed along a helical path surrounding the laser-accelerated ion beams, addresses these shortcomings simultaneously. In a proof-of-principle experiment on a university-scale system, we demonstrate post-acceleration of laser-driven protons from a flat foil at a rate of 0.5 GeV m−1, already beyond what can be sustained by conventional accelerator technologies, with dynamic beam collimation and energy selection. These results open up new opportunities for the development of extremely compact and cost-effective ion accelerators for both established and innovative applications. PMID:27089200

  7. Guided post-acceleration of laser-driven ions by a miniature modular structure.

    PubMed

    Kar, Satyabrata; Ahmed, Hamad; Prasad, Rajendra; Cerchez, Mirela; Brauckmann, Stephanie; Aurand, Bastian; Cantono, Giada; Hadjisolomou, Prokopis; Lewis, Ciaran L S; Macchi, Andrea; Nersisyan, Gagik; Robinson, Alexander P L; Schroer, Anna M; Swantusch, Marco; Zepf, Matt; Willi, Oswald; Borghesi, Marco

    2016-01-01

    All-optical approaches to particle acceleration are currently attracting a significant research effort internationally. Although characterized by exceptional transverse and longitudinal emittance, laser-driven ion beams currently have limitations in terms of peak ion energy, bandwidth of the energy spectrum and beam divergence. Here we introduce the concept of a versatile, miniature linear accelerating module, which, by employing laser-excited electromagnetic pulses directed along a helical path surrounding the laser-accelerated ion beams, addresses these shortcomings simultaneously. In a proof-of-principle experiment on a university-scale system, we demonstrate post-acceleration of laser-driven protons from a flat foil at a rate of 0.5 GeV m(-1), already beyond what can be sustained by conventional accelerator technologies, with dynamic beam collimation and energy selection. These results open up new opportunities for the development of extremely compact and cost-effective ion accelerators for both established and innovative applications. PMID:27089200

  8. Laser system for Doppler cooling of ytterbium ion in an optical frequency standard

    NASA Astrophysics Data System (ADS)

    Chepurov, S. V.; Lugovoy, A. A.; Kuznetsov, S. N.

    2014-06-01

    A laser system for Doppler cooling of ytterbium ion on the 2S1/2 → 2P1/2 transition in a single-ion optical frequency standard is developed. The second harmonic of a semiconductor laser with a wavelength of 739 nm is used for cooling. The laser frequency is doubled in a nonlinear BiBO crystal embedded in a ring resonator, which also serves as a reference for laser frequency stabilisation. Second-harmonic power of ~100 μW is generated at a wavelength of 369.5 nm. Diode laser radiation is modulated by an electro-optic modulator at 14.75 GHz to generate a sideband exciting the 2S1/2 (F = 0) → 2P1/2 (F = 1) hyperfine component of the cooling transition that is not excited by resonant cooling light. The sideband relative intensity of a few percent proved to be sufficient to reduce the ion dwelling time in the 2S1/2 (F = 0) state to less than 10-4 s and increase the cooling efficiency.

  9. Laser system for Doppler cooling of ytterbium ion in an optical frequency standard

    SciTech Connect

    Chepurov, S V; Lugovoy, A A; Kuznetsov, S N

    2014-06-30

    A laser system for Doppler cooling of ytterbium ion on the {sup 2}S{sub 1/2} → {sup 2}P{sub 1/2} transition in a single-ion optical frequency standard is developed. The second harmonic of a semiconductor laser with a wavelength of 739 nm is used for cooling. The laser frequency is doubled in a nonlinear BiBO crystal embedded in a ring resonator, which also serves as a reference for laser frequency stabilisation. Second-harmonic power of ∼100 μW is generated at a wavelength of 369.5 nm. Diode laser radiation is modulated by an electro-optic modulator at 14.75 GHz to generate a sideband exciting the {sup 2}S{sub 1/2} (F = 0) → {sup 2}P{sub 1/2} (F = 1) hyperfine component of the cooling transition that is not excited by resonant cooling light. The sideband relative intensity of a few percent proved to be sufficient to reduce the ion dwelling time in the {sup 2}S{sub 1/2} (F = 0) state to less than 10{sup -4} s and increase the cooling efficiency. (extreme light fields and their applications)

  10. Detection of explosive related nitroaromatic compounds (ERNC) by laser-based ion mobility spectrometry

    NASA Astrophysics Data System (ADS)

    Laudien, Robert; Riebe, Daniel; Beitz, Toralf; Löhmannsröben, Hans-Gerd

    2008-10-01

    In this study two issues are addressed, namely laser ionisation of selected nitroaromatic compounds (NAC) and the characterisation of their anions by photodetachment (PD) spectroscopy. Laser ionisation of the NAC at λ = 226.75 nm is investigated by ion mobility (IM) spectrometry at atmospheric pressure. The main product after laser ionisation is the reactive NO+ ion formed in a sequence of photofragmentation and multiphoton ionisation processes. NO+ is trapped by specific ion molecule reactions (IMR). Alternatively, NO, added as laser dopant, can directly be ionised. The formed NO+ reacts with the NAC under complex formation. This allows fragmentless NAC detection. The combination of IM spectrometry and PD spectroscopy provides real-time characterisation of the anions in the IM spectrum. This is useful to differentiate between NAC and interfering substances and, thus, to reduce false-positive detections of NAC. The electrons detached by the PD laser at λ = 532 nm are detected in the same spectrum as the anions. The potential of PD-IM spectrometry in terms of cross section determination, analytical improvements, tomographic mapping, spatial hole burning etc., is outlined.

  11. Formation and fragmentation of quadruply charged molecular ions by intense femtosecond laser pulses.

    PubMed

    Yatsuhashi, Tomoyuki; Nakashima, Nobuaki

    2010-07-22

    We investigated the formation and fragmentation of multiply charged molecular ions of several aromatic molecules by intense nonresonant femtosecond laser pulses of 1.4 mum with a 130 fs pulse duration (up to 2 x 10(14) W cm(-2)). Quadruply charged states were produced for 2,3-benzofluorene and triphenylene molecular ion in large abundance, whereas naphthalene and 1,1'-binaphthyl resulted only in up to triply charged molecular ions. The laser wavelength was nonresonant with regard to the electronic transitions of the neutral molecules, and the degree of fragmentation was strongly correlated with the absorption of the singly charged cation radical. Little fragmentation was observed for naphthalene (off-resonant with cation), whereas heavy fragmentation was observed in the case of 1,1'-binaphthyl (resonant with cation). The degree of H(2) (2H) and 2H(2) (4H) elimination from molecular ions increased as the charge states increased in all the molecules examined. A striking difference was found between triply and quadruply charged 2,3-benzofluorene: significant suppression of molecular ions with loss of odd number of hydrogen was observed in the quadruply charged ions. The Coulomb explosion of protons in the quadruply charged state and succeeding fragmentation resulted in the formation of triply charged molecular ions with an odd number of hydrogens. The hydrogen elimination mechanism in the highly charged state is discussed.

  12. Formation and fragmentation of quadruply charged molecular ions by intense femtosecond laser pulses.

    PubMed

    Yatsuhashi, Tomoyuki; Nakashima, Nobuaki

    2010-07-22

    We investigated the formation and fragmentation of multiply charged molecular ions of several aromatic molecules by intense nonresonant femtosecond laser pulses of 1.4 mum with a 130 fs pulse duration (up to 2 x 10(14) W cm(-2)). Quadruply charged states were produced for 2,3-benzofluorene and triphenylene molecular ion in large abundance, whereas naphthalene and 1,1'-binaphthyl resulted only in up to triply charged molecular ions. The laser wavelength was nonresonant with regard to the electronic transitions of the neutral molecules, and the degree of fragmentation was strongly correlated with the absorption of the singly charged cation radical. Little fragmentation was observed for naphthalene (off-resonant with cation), whereas heavy fragmentation was observed in the case of 1,1'-binaphthyl (resonant with cation). The degree of H(2) (2H) and 2H(2) (4H) elimination from molecular ions increased as the charge states increased in all the molecules examined. A striking difference was found between triply and quadruply charged 2,3-benzofluorene: significant suppression of molecular ions with loss of odd number of hydrogen was observed in the quadruply charged ions. The Coulomb explosion of protons in the quadruply charged state and succeeding fragmentation resulted in the formation of triply charged molecular ions with an odd number of hydrogens. The hydrogen elimination mechanism in the highly charged state is discussed. PMID:20578764

  13. Enabling coherent control of trapped ions with economical multi-laser frequency stabilization technology

    NASA Astrophysics Data System (ADS)

    Lybarger, Warren Emanuel, Jr.

    A phase-locked scanning stability transfer cavity (SSTC) for transferring the absolute frequency stability of an iodine referenced He-Ne (master) laser to three otherwise uncalibrated (slave) lasers (at 844, 1033, & 1092 nm) of a trapped-Sr+ quantum information processing (QIP) apparatus is described. When locked, the 422 nm frequency-doubled Doppler-cooling laser exhibits an error of <1 MHz RMS for several hours, and similar stability is achieved with the other slave lasers. When unlocked, each slave laser drifts by a large fraction (or more) of the corresponding transition linewidth in minutes, thus making reliable laser cooling, ion state readout, and execution of QIP algorithms practically infeasible. The SSTC makes coherent control of Sr+ possible by addressing this problem, and the QIP apparatus is now sufficiently stable for single user operation. New single-ion experimental capabilities include ground state cooling, high-fidelity Rabi flopping, Ramsey interferometry, and sympathetic cooling of 88Sr+( 86Sr+) with 86Sr+( 88Sr+). A 2.5 msec coherence time has been achieved with the optical quoit encoded in a |5 2S 1/2> ↔ |4 2D5/2> quadrupole transition, a precision measurement of the isotope shift of the qubit transition in 86Sr+ relative to 88Sr+ is reported, and a single-ion heating rate consistent with results throughout the trapped-ion community is reported. The SSTC is simple to implement, uses no custom optics, and it has a higher scanning rate than previously demonstrated SSTC's. Phase-locked SSTC's are shown to have an advantage over the more common displacement-locked SSTC in the low finesse regime, and they are an attractive alternative to passively stable but complex optical references and diode lasers designed to address the same problem. The SSTC is useful in spectroscopic applications with other ion species, atoms, and molecules, in general. An appendix is dedicated to describing in detail an advanced trapped-ion quantum processor concept

  14. Laser-Accelerated Ions from a Shock-Compressed Gas Foil

    NASA Astrophysics Data System (ADS)

    Helle, M. H.; Gordon, D. F.; Kaganovich, D.; Chen, Y.; Palastro, J. P.; Ting, A.

    2016-10-01

    We present results of energetic laser-ion acceleration from a tailored, near solid density gas target. Colliding hydrodynamic shocks compress a pure hydrogen gas jet into a 70 μ m thick target prior to the arrival of the ultraintense laser pulse. A density scan reveals the transition from a regime characterized by a wide angle, low-energy beam (target normal sheath acceleration) to one of a more focused beam with a high-energy halo (magnetic vortex acceleration). In the latter case, three-dimensional simulations show the formation of a Z pinch driven by the axial current resulting from laser wakefield accelerated electrons. Ions at the rear of the target are then accelerated by a combination of space charge fields from accelerated electrons and Coulombic repulsion as the pinch dissipates.

  15. A comprehensive study on the laser decontamination of surfaces contaminated with Cs(+) ion.

    PubMed

    Baigalmaa, B; Won, H J; Moon, J K; Jung, C H; Hyun, J H

    2009-01-01

    A Q-switched Nd:YAG laser with a 1064nm, 450mJ/pulse and 14ns pulse width was employed to study the decontamination characteristics of Type 304 stainless steel specimens contaminated with Cs(+) ions. The surrogate specimens were artificially contaminated with two kinds of premixed solutions. The laser was irradiated for 10, 20 and 100 shots. The results were investigated using a SEM, EPMA and XPS. For the surrogate specimen treated with the CsCl+KCl solution, more than 98% of the Cs(+) ions were removed during an irradiation of 100 shots. The specimen treated with the CsCl+KCl solution was easier to decontaminate. By comparing the ratio of the O(1s) intensity to the Fe(2p) intensity of the XPS spectra, it was found that the oxygen atoms that had evolved from the specimen treated with the CsNO(3)+KNO(3) solution had decreased the laser's decontamination performance.

  16. Energy gain and spectral tailoring of ion beams using ultra-high intensity laser beams

    NASA Astrophysics Data System (ADS)

    Prasad, Rajendra; Swantusch, Marco; Cerchez, Mirela; Spickermann, Sven; Auorand, Bastian; Wowra, Thomas; Boeker, Juergen; Willi, Oswald

    2015-11-01

    The field of laser driven ion acceleration over the past decade has produced a huge amount of research. Nowadays, several multi-beam facilities with high rep rate system, e.g. ELI, are being developed across the world for different kinds of experiments. The study of interaction dynamics of multiple beams possessing ultra-high intensity and ultra-short pulse duration is of vital importance. Here, we present the first experimental results on ion acceleration using two ultra-high intensity beams. Thanks to the unique capability of Arcturus laser at HHU Düsseldorf, two almost identical, independent beams in laser parameters such as intensity (>1020 W/cm2), pulse duration (30 fs) and contrast (>1010), could be accessed. Both beams are focused onto a 5 μm thin Ti target. While ensuring spatial overlap of the two beams, at relative temporal delay of ~ 50 ps (optimum delay), the proton and carbon ion energies were enhanced by factor of 1.5. Moreover, strong modulation in C4+ions near the high energy cut-off is observed later than the optimum delay for the proton enhancement. This offers controlled tailoring of the spectral content of heavy ions.

  17. Picosecond ion pulses from an EN tandem created by a femtosecond Ti:sapphire laser

    NASA Astrophysics Data System (ADS)

    Carnes, K. D.; Cocke, C. L.; Chang, Z.; Ben-Itzhak, I.; Needham, H. V.; Rankin, A.

    2007-08-01

    As the James R. Macdonald Laboratory at Kansas State University continues its transformation from an ion collisions facility to an ultrafast laser/ion collisions facility, we are looking for novel ways to combine our traditional accelerator expertise with our new laser capabilities. One such combination is to produce picosecond pulses of stripping gas ions in the high energy accelerating tube of our EN tandem by directing ∼100 fs, sub-milliJoule laser pulses up the high energy end of the tandem toward a focusing mirror at the terminal. Ion pulses from both stripping and residual gas have been produced and identified, with pulse widths thus far on the order of a nanosecond. This width represents an upper limit, as it is dominated by pulse-to-pulse jitter in the ion time-of-flight (TOF) and is therefore not a true representation of the actual pulse width. In this paper, we describe the development process and report on the results to date. Conditions limiting the minimum temporal pulse width, such as tandem terminal ripple, thermal motion of the gas and space charge effects, are also outlined.

  18. Resonant laser ablation ion trap mass spectrometry -- Recent applications for chemical analysis

    SciTech Connect

    Gill, C.G.; Garrett, A.W.; Hemberger, P.H.; Nogar, N.S.

    1995-12-31

    Resonant Laser Ablation (RLA) is a useful ionization process for selectively producing gas phase ions from a solid sample. Recent use of RLA for mass spectrometry by this group and by others has produced a wealth of knowledge and useful analytical techniques. The method relies upon the focusing of modest intensity laser pulses ({le} 10{sup 7} W {center_dot} Cm{sup {minus}2}) upon a sample surface. A small quantity of material is vaporized, and atoms of desired analyte are subsequently ionized by (n + m) photon processes in the gas phase (where n = number of photons to a resonant transition and m = number of photons to exceed the ionization limit). The authors have been using (2 + 1) resonant ionization schemes for this work. Quadrupole ion trap mass spectrometry is realizing a very prominent role in current mass spectrometric research. Ion traps are versatile, powerful and extremely sensitive mass spectrometers, capable of a variety of ionization modes, MS{sup n} type experiments, high mass ranges and high resolution, all for a fraction of the cost of other instrumentation with similar capabilities. Quadrupole ion traps are ideally suited to pulsed ionization sources such as laser ionization methods, since their normal operational method (Mass Selective Instability) relies upon the storage of ions from a finite ionization period followed by ejection and detection of these ions based upon their mass to charge ratios. The paper describes selective ionization for trace atomic analysis, selective reagent ion source for ion chemistry investigations, and the analysis of ``difficult`` environmental contaminants, i.e., TBP.

  19. Increased efficiency of ion acceleration by using femtosecond laser pulses at higher harmonic frequency

    SciTech Connect

    Psikal, J.; Klimo, O.; Weber, S.; Margarone, D.

    2014-07-15

    The influence of laser frequency on laser-driven ion acceleration is investigated by means of two-dimensional particle-in-cell simulations. When ultrashort intense laser pulse at higher harmonic frequency irradiates a thin solid foil, the target may become re lativistically transparent for significantly lower laser pulse intensity compared with irradiation at fundamental laser frequency. The relativistically induced transparency results in an enhanced heating of hot electrons as well as increased maximum energies of accelerated ions and their numbers. Our simulation results have shown the increase in maximum proton energy and increase in the number of high-energy protons by a factor of 2 after the interaction of an ultrashort laser pulse of maximum intensity 7 × 10{sup 21 }W/cm{sup 2} with a fully ionized plastic foil of realistic density and of optimal thickness between 100 nm and 200 nm when switching from the fundamental frequency to the third harmonics.

  20. Investigation of efficient shock acceleration of ions using high energy lasers in low density targets

    NASA Astrophysics Data System (ADS)

    Antici, P.; Gauthier, M.; D'Humieres, E.; Albertazzi, B.; Beaucourt, C.; Böker, J.; Chen, S.; Dervieux, V.; Feugeas, J. L.; Glesser, M.; Levy, A.; Nicolai, P.; Romagnani, L.; Tikhonchuk, V.; Pepin, H.; Fuchs, J.

    2012-10-01

    Intense research is being conducted on sources of laser-accelerated ions and their applications that have the potential of becoming novel particle sources. In most experiments, a high intensity and short laser pulse interacts with a solid density target. It was recently shown that a promising way to accelerate ions to higher energies and in a collimated beam is to use under-dense or near-critical density targets instead of solid ones. In these conditions, simulations have revealed that protons are predicted to be accelerated by a collisionless shock mechanism that significantly increases their energy. We present recent experiments performed on the 100 TW LULI laser (France) and the TITAN facility at LLNL, USA. The near critical density plasma was prepared by exploding thin solid foils by a long laser pulse. The plasma density profile was controlled by varying the target thickness and the delay between the long and the short laser pulse. When exploding the target, we obtained proton energies that are comparable if not higher than what was obtained under similar laser conditions, but with solid targets which make them a promising candidate for an efficient proton source.

  1. Measurement of xenon plasma properties in an ion thruster using laser Thomson scattering technique

    SciTech Connect

    Yamamoto, N.; Tomita, K.; Sugita, K.; Kurita, T.; Nakashima, H.; Uchino, K.

    2012-07-15

    This paper reports on the development of a method for measuring xenon plasma properties using the laser Thomson scattering technique, for application to ion engine system design. The thresholds of photo-ionization of xenon plasma were investigated and the number density of metastable atoms, which are photo-ionized by a probe laser, was measured using laser absorption spectroscopy, for several conditions. The measured threshold energy of the probe laser using a plano-convex lens with a focal length of 200 mm was 150 mJ for a xenon mass flow rate of 20 {mu}g/s and incident microwave power of 6 W; the probe laser energy was therefore set as 80 mJ. Electron number density was found to be (6.2 {+-} 0.4) Multiplication-Sign 10{sup 17} m{sup -3} and electron temperature was found to be 2.2 {+-} 0.4 eV at a xenon mass flow rate of 20 {mu}g/s and incident microwave power of 6 W. The threshold of the probe laser intensity against photo-ionization in a miniature xenon ion thruster is almost constant for various mass flow rates, since the ratio of population of the metastable atoms to the electron number density is little changed.

  2. Ion Emission Characteristics of a Forward Laser Accelerated Plasma Thruster

    SciTech Connect

    Oyaizu, Keishi; Izumi, Masaya; Horisawa, Hideyuki; Kimura, Itsuro

    2005-04-27

    A fundamental study of a forward laser accelerated plasma thruster was conducted. In order to evaluate thrust performances of the thruster, a time-of-flight measurement was conducted for an Al-foil target irradiated with an Nd:YAG laser of 1J/pulse with pulse-width of 10nsec. From the measurement, the average plasma speed was about 53 km/sec. Time-gated imaging of the plasma with an ICCD camera was also conducted. From the observation, rapid plasmas were observed on both sides of the target. Each image from the ICCD camera was processed by an image processing software into an emission intensity distribution of the plasma at every 10nsec. Axial velocity of the plasma was estimated from the temporal evolution of the plasma edge. The average and maximum plasma expansion velocities in a forward direction were estimated about 40 km/s and 160 km/sec, respectively.

  3. Laser ion acceleration by a near-critical density target

    SciTech Connect

    Yogo, A.; Daido, H.; Bulanov, S. V.; Esirkepov, T. Zh.; Ogura, K.; Orimo, S.; Sagisaka, A.; Ma, J.-L.; Mori, M.; Nishiuchi, M.; Pirozhkov, A. S.; Nemoto, K.; Oishi, Y.; Nayuki, T.; Fujii, T.; Nakamura, S.; Noda, A.; Nagatomo, H.

    2008-06-24

    Protons having energies up to 3.8 MeV are experimentally generated by the p-polarized, 45 fs, {approx}10{sup 19} W/cm{sup 2} laser pulse interacting with a near-critical plasma cloud produced by the irradiation of the amplified spontaneous emission (ASE) pedestal at an intensity of {approx}10{sup 13} W/cm{sup 2} onto a 7.5-{mu}m-thick polyimide foil target. The emission angle of the high-energy protons is shifted away from the target normal toward the laser-propagation direction of 45 deg. The mechanism which explains the proton generation from the near-critical plasma cloud is discussed using the two-dimensional (2D) particle-in-cell (PIC) simulation.

  4. Emittance dependence on anode morphology of an ion beam provided by laser ablation

    NASA Astrophysics Data System (ADS)

    Velardi, L.; Delle Side, D.; Nassisi, V.

    2014-07-01

    In this work, we studied the characteristics of ion beams generated by Platone accelerator in different anode configurations. The accelerator is a laser ion source with two gaps which accelerate the ions in cascade. The laser is a ns pulsed KrF able to apply irradiances of 109-1010 W/cm2. The target ablated was pure disk of Cu. The accelerating voltage applied in this work was 60 kV. The emittance evaluation was performed by the pepper pot method utilizing radio-chromic films, EBT Gafchromic, as sensible targets. The study was performed by varying the geometric configuration of the anode (the extracting electrode), modifying the hole morphology, e.g. a plane and curved grid were mounted in order to change the extraction configuration. The results were compared with the ones obtained with the extraction hole without any grid. For the normalized emittance the lowest value was 0.20π mm mrad.

  5. On the Emittance dependence on anode morphology of laser induced ion beams

    NASA Astrophysics Data System (ADS)

    Velardi, L.; Delle Side, D.; Nassisi, V.

    2014-04-01

    In this work, we studied the characteristics of ion beams generated by PLATONE accelerator in different anode configurations. The accelerator is a laser ion source with two gaps which accelerate the ions in cascade. The laser is an excimer KrF able to work at irradiances of 108-1010 W/cm2. The target ablated was disk of Cu. The accelerating voltage applied in this work was 60 kV. The emittance evaluation was performed by the pepper pot method utilising radio-chromic films, EBT Gafchromic, as sensible targets. The study was performed by varying the geometric configuration of the anode (the extracting electrode), modifying the hole morphology. A plane and curved grids were mounted in order to change the extraction configuration. The results were compared with the ones obtained with the extraction hole without any grid. For the normalized emittance the lowest value found was 0.20 π mm mrad.

  6. Comparison of Single Event Transients Generated by Short Pulsed X-Rays, Lasers and Heavy Ions

    SciTech Connect

    Cardoza, David; LaLumondiere, Stephen D.; Tockstein, Michael A.; Brewe, Dale L.; Wells, Nathan P.; Koga, Rokutaro; Gaab, K. M.; Lotshaw, William T.; Moss, Steven C.

    2014-12-01

    We report an experimental study of the transients generated by pulsed x-rays, heavy ions, and different laser wavelengths in a Si p-i-n photodiode. We compare the charge collected by all of the excitation methods to determine the equivalent LET for pulsed x-rays relative to heavy ions. Our comparisons show that pulsed x-rays from synchrotron sources can generate a large range of equivalent LET and generate transients similar to those excited by laser pulses and heavy ion strikes. We also look at how the pulse width of the transients changes for the different excitation methods. We show that the charge collected with pulsed x-rays is greater than expected as the x-ray photon energy increases. Combined with their capability of focusing to small spot sizes and of penetrating metallization, pulsed x-rays are a promising new tool for high resolution screening of SEE susceptibility

  7. Ion intensity and thermal proton transfer in ultraviolet matrix-assisted laser desorption/ionization.

    PubMed

    Lu, I-Chung; Lee, Chuping; Chen, Hui-Yuan; Lin, Hou-Yu; Hung, Sheng-Wei; Dyakov, Yuri A; Hsu, Kuo-Tung; Liao, Chih-Yu; Lee, Yin-Yu; Tseng, Chien-Ming; Lee, Yuan-Tseh; Ni, Chi-Kung

    2014-04-17

    The ionization mechanism of ultraviolet matrix-assisted laser desorption/ionization (UV-MALDI) was investigated by measuring the total cation intensity (not including sodiated and potasiated ions) as a function of analyte concentration (arginine, histidine, and glycine) in a matrix of 2,4,6-trihydroxyacetophenone (THAP). The total ion intensity increased up to 55 times near the laser fluence threshold as the arginine concentration increased from 0% to 1%. The increases were small for histidine, and a minimal increase occurred for glycine. Time-resolved fluorescence intensity was employed to investigate how analytes affected the energy pooling of the matrix. No detectable energy pooling was observed for pure THAP and THAP/analyte mixtures. The results can be described by using a thermal proton transfer model, which suggested that thermally induced proton transfer is crucial in the primary ion generation in UV-MALDI.

  8. Ion Acceleration by Laser Plasma Interaction from Cryogenic Micro Jets - Oral Presentation

    SciTech Connect

    Propp, Adrienne

    2015-08-25

    Processes that occur in extreme conditions, such as in the center of stars and large planets, can be simulated in the laboratory using facilities such as SLAC National Accelerator Laboratory and the Jupiter Laser Facility (JLF) at Lawrence Livermore National Laboratory (LLNL). These facilities allow scientists to investigate the properties of matter by observing their interactions with high power lasers. Ion acceleration from laser plasma interaction is gaining greater attention today due to its widespread potential applications, including proton beam cancer therapy and fast ignition for energy production. Typically, ion acceleration is achieved by focusing a high power laser on thin foil targets through a mechanism called Target Normal Sheath Acceleration. Based on research and recent experiments, we hypothesized that a pure liquid cryogenic jet would be an ideal target for this type of interaction, capable of producing the highest proton energies possible with today’s laser technologies. Furthermore, it would provide a continuous, pure target, unlike metal foils which are consumed in the interaction and easily contaminated. In an effort to test this hypothesis and investigate new, potentially more efficient mechanisms of ion acceleration, we used the 527 nm split beam, frequency-doubled TITAN laser at JLF. Data from the cryogenic jets was limited due to the flow of current up the jet into the nozzle during the interaction, heating the jet and damaging the orifice. However, we acheived a pure proton beam with an indiciation of a monoenergetic feature. Furthermore, data from gold and carbon wires showed surprising and interesting results. Preliminary analysis of data from two ion emission diagnostics, Thomson parabola spectrometers (TPs) and radio chromic films (RCFs), suggests that shockwave acceleration occurred rather than target normal sheath acceleration, the standard mechanism of ion acceleration. Upon completion of the experiment at TITAN, I researched the

  9. Ion acceleration from the interaction of ultra-intense lasers with solid foils

    NASA Astrophysics Data System (ADS)

    Allen, Matthew Mark

    The discovery that ultra-intense laser pulses (I > 10 18 W/cm2) can produce short pulse, high energy proton beams has renewed interest in the fundamental mechanisms that govern particle acceleration from laser-solid interactions. In this thesis we present several experiments that study the accelerated ions by affecting the contamination layer from which they originate. Radiative heating was employed as a method of removing contamination from palladium targets doped with deuterium. We present evidence that ions heavier than protons can be accelerated if hydrogenous contaminants that cover the laser target can be removed. We show that deuterons can be accelerated from the deuterated-palladium target, which has been radiatively heating to remove contaminants. Impinging a deuteron beam onto a tritiated-titanium catcher could lead to the development of a table-top source of short-pulse, 14-MeV fusion neutrons. We also show that by using an argon-ion sputter gun, contaminants from one side of the laser target can be selectively removed without affecting the other side. We show that irradiating a thin metallic foil with an ultra-intense laser pulse produces a proton beam with a yield of 1.5--2.5 10 11 and temperature, kT = 1.5 MeV with a maximum proton energy >9 MeV. Removing contaminants from the front surface of the laser target with an argon-ion sputter gun, had no observable effect on the proton beam. However, removing contaminants from the back surface of the laser target reduced the proton beam by two orders of magnitude to, at most, a yield of ˜10 9 and a maximum proton energy <4 MeV. Based on these observations, we conclude that the majority (>99%) of high energy protons (E > 5 MeV) from the interaction of an ultra-intense laser pulse with a thin foil originate on the back surface of the foil---as predicted by the TNSA model. Our experimental results are in agreement with PIC simulations showing back surface protons reach energies up to 13 MeV, while front

  10. High-intensity laser-accelerated ion beam produced from cryogenic micro-jet target

    NASA Astrophysics Data System (ADS)

    Gauthier, M.; Kim, J. B.; Curry, C. B.; Aurand, B.; Gamboa, E. J.; Göde, S.; Goyon, C.; Hazi, A.; Kerr, S.; Pak, A.; Propp, A.; Ramakrishna, B.; Ruby, J.; Willi, O.; Williams, G. J.; Rödel, C.; Glenzer, S. H.

    2016-11-01

    We report on the successful operation of a newly developed cryogenic jet target at high intensity laser-irradiation. Using the frequency-doubled Titan short pulse laser system at Jupiter Laser Facility, Lawrence Livermore National Laboratory, we demonstrate the generation of a pure proton beam a with maximum energy of 2 MeV. Furthermore, we record a quasi-monoenergetic peak at 1.1 MeV in the proton spectrum emitted in the laser forward direction suggesting an alternative acceleration mechanism. Using a solid-density mixed hydrogen-deuterium target, we are also able to produce pure proton-deuteron ion beams. With its high purity, limited size, near-critical density, and high-repetition rate capability, this target is promising for future applications.

  11. Spectra of multiply charged hollow ions in the plasma produced by a short-wavelength nanosecond laser

    SciTech Connect

    Abdallah, J; Skobelev, I Yu; Faenov, A Ya; Magunov, A I; Pikuz, T A; Flora, F; Bollanti, S; DiLazzaro, P; Letardi, T; Burattini, E; Grilli, A; Reale, A; Palladino, L; Tomassetti, G; Scafati, A; Reale, L

    2000-08-31

    Complex spectral structures located between the resonance lines of H- and He-like MgXII and MgXI ions were recorded in experiments on plasma heating by the radiation of a low-power short-wavelength excimer XeCl laser (12-ns pulses with an energy of 2 J). The above spectral structures were shown to arise from transitions in the so-called hollow multicharged ions, i.e., in ions with an empty 1s-shell, which were previously observed in laser produced plasmas only with ultrahigh-power femto- and picosecond laser facilities having extremely high-contrast laser pulses. (interaction of laser radiation with matter. laser plasma)

  12. Uniform heating of materials into the warm dense matter regime with laser-driven quasimonoenergetic ion beams

    SciTech Connect

    Bang, W.; Albright, B. J.; Bradley, P. A.; Vold, E. L.; Boettger, J. C.; Fernández, J. C.

    2015-12-01

    In a recent experiment at the Trident laser facility, a laser-driven beam of quasimonoenergetic aluminum ions was used to heat solid gold and diamond foils isochorically to 5.5 and 1.7 eV, respectively. Here theoretical calculations are presented that suggest the gold and diamond were heated uniformly by these laser-driven ion beams. According to calculations and SESAME equation-of-state tables, laser-driven aluminum ion beams achievable at Trident, with a finite energy spread of ΔE/E~20%, are expected to heat the targets more uniformly than a beam of 140-MeV aluminum ions with zero energy spread. As a result, the robustness of the expected heating uniformity relative to the changes in the incident ion energy spectra is evaluated, and expected plasma temperatures of various target materials achievable with the current experimental platform are presented.

  13. Uniform heating of materials into the warm dense matter regime with laser-driven quasimonoenergetic ion beams

    DOE PAGES

    Bang, W.; Albright, B. J.; Bradley, P. A.; Vold, E. L.; Boettger, J. C.; Fernández, J. C.

    2015-12-01

    In a recent experiment at the Trident laser facility, a laser-driven beam of quasimonoenergetic aluminum ions was used to heat solid gold and diamond foils isochorically to 5.5 and 1.7 eV, respectively. Here theoretical calculations are presented that suggest the gold and diamond were heated uniformly by these laser-driven ion beams. According to calculations and SESAME equation-of-state tables, laser-driven aluminum ion beams achievable at Trident, with a finite energy spread of ΔE/E~20%, are expected to heat the targets more uniformly than a beam of 140-MeV aluminum ions with zero energy spread. As a result, the robustness of the expected heatingmore » uniformity relative to the changes in the incident ion energy spectra is evaluated, and expected plasma temperatures of various target materials achievable with the current experimental platform are presented.« less

  14. INTERACTION OF LASER RADIATION WITH MATTER. LASER PLASMA: Influence of corundum structure on the characteristics of multiply charged ions in a laser-produced plasma

    NASA Astrophysics Data System (ADS)

    Bedilov, M. R.; Beisembaeva, Kh B.; Sabitov, M. S.

    2000-01-01

    An investigation was made of the interaction of intense laser radiation (λ = 1.06 μm) with previously irradiated corundum. The studies were performed in the collecting mode by employing time-of-flight mass spectrometry. Electron and ion currents were considered simultaneously with charge-state and energy characteristics of multiply charged ions of the plasmas produced at the source and previously irradiated targets. The combined consideration allows the conclusion that the prior neutron irradiation of a sample by a fluence of 1015 — 1019 neutron cm-2 makes for production of a higher-temperature plasma.

  15. Direct spectroscopic observation of ion deceleration accompanying laser plasma-wall interaction

    NASA Astrophysics Data System (ADS)

    Renner, O.; Krouský, E.; Liska, R.; Šmíd, M.; Larroche, O.; Dalimier, E.; Rosmej, F. B.

    2010-08-01

    Interactions of plasma jets with solid surfaces are extensively studied in context with development of future fusion devices. In experiments carried out on the iodine laser system PALS, the energetic ions were produced at double-foil Al/Mg targets irradiated by one or two counter-propagating laser beams. The plasma jets from the rear surface of the laser-exploded Al foil streamed towards the Mg target representing the wall preheated by the action of the high-energy photons, particle and/or laser beams. Instead of being trapped by the cold secondary-target material, the forward-accelerated Al ions collided with the counter-propagating matter ejected from the wall. The environmental conditions in near-wall plasmas were analyzed with the high-resolution x-ray spectroscopy and temporally-resolved x-ray imaging. The deceleration of the incident Al ions in the near-wall region was directly observed and quantitatively characterized via Doppler shifts of the J-satellite from the Al Lya spectral group. The interaction scenario was modelled using the 2D arbitrary Lagrangian Eulerian hydrocode PALE and the multifluid code MULTIF.

  16. Gaussian energy distribution of fast ions emitted by laser-produced plasmas

    NASA Astrophysics Data System (ADS)

    Krása, J.

    2013-05-01

    The analysis of ion collector signals with the use of a time-of-fight signal function derived from a shifted Maxwell-Boltzmann velocity distribution is used to quantify the ion characteristics as the ion temperature and velocity of centre-of-mass motion of groups of ionized species constituting the ablated plasma. The analysis is also focused on velocity and energy distributions derived from the signal of a time-of-flight detector taking into account the underlying principle of sensor operation. The energy Maxwell spectra of ions are compared with the Gauss distribution with respect to the ratio of the centre-of-mass energy of ions to their temperature. The difference threshold between the Gauss and energy Maxwell spectra is determined via the limited validity of the basic relationship between spreads in energy and time-of-flight spectra ½ΔE/E = Δt/t. The analysis of velocity spectrum of fast ions emitted by Ti plasma produced with 300 ps, kJ-class iodine laser operating at PALS facility shows that ion bursts consist of almost monoenergetic ion beams.

  17. In situ mitigation of subsurface and peripheral focused ion beam damage via simultaneous pulsed laser heating

    DOE PAGES

    Stanford, Michael G.; Lewis, Brett B.; Iberi, Vighter O.; Fowlkes, Jason Davidson; Tan, Shida; Livengood, Rick; Rack, Philip D.

    2016-02-16

    Focused helium and neon ion (He(+)/Ne(+) ) beam processing has recently been used to push resolution limits of direct-write nanoscale synthesis. The ubiquitous insertion of focused He(+) /Ne(+) beams as the next-generation nanofabrication tool-of-choice is currently limited by deleterious subsurface and peripheral damage induced by the energetic ions in the underlying substrate. The in situ mitigation of subsurface damage induced by He(+)/Ne(+) ion exposures in silicon via a synchronized infrared pulsed laser-assisted process is demonstrated. The pulsed laser assist provides highly localized in situ photothermal energy which reduces the implantation and defect concentration by greater than 90%. The laser-assisted exposuremore » process is also shown to reduce peripheral defects in He(+) patterned graphene, which makes this process an attractive candidate for direct-write patterning of 2D materials. In conclusion, these results offer a necessary solution for the applicability of high-resolution direct-write nanoscale material processing via focused ion beams.« less

  18. Laser-induced fluorescence from N2(+) ions generated by a corona discharge in ambient air.

    PubMed

    Konthasinghe, Kumarasiri; Fitzmorris, Kristin; Peiris, Manoj; Hopkins, Adam J; Petrak, Benjamin; Killinger, Dennis K; Muller, Andreas

    2015-09-01

    In this work, we present the measurement of laser-induced fluorescence from N2(+) ions via the B(2)Σu(+)-X(2)Σg(+) band system in the near-ultraviolet. The ions were generated continuously by a plasma glow discharge in low pressure N2 and by a corona discharge in ambient air. The fluorescence decay time was found to rapidly decrease with increasing pressure leading to an extrapolated decay rate of ≍10(10) s(-1) at atmospheric pressure. In spite of this quenching, we were able to observe laser induced fluorescence in ambient air by means of a time-gated spectral measurement. In the process of comparing the emission signal with that of N2 spontaneous Raman scattering, ion concentrations in ambient air of order 10(8-)10(10) cm(-3) were determined. With moderate increases in laser power and collection efficiency, ion concentrations of less than 10(6) cm(-3) may be measurable, potentially enabling applications in atmospheric standoff detection of ionizing radiation from hazardous radioactive sources. PMID:26414524

  19. In Situ Mitigation of Subsurface and Peripheral Focused Ion Beam Damage via Simultaneous Pulsed Laser Heating.

    PubMed

    Stanford, Michael G; Lewis, Brett B; Iberi, Vighter; Fowlkes, Jason D; Tan, Shida; Livengood, Rick; Rack, Philip D

    2016-04-01

    Focused helium and neon ion (He(+)/Ne(+)) beam processing has recently been used to push resolution limits of direct-write nanoscale synthesis. The ubiquitous insertion of focused He(+)/Ne(+) beams as the next-generation nanofabrication tool-of-choice is currently limited by deleterious subsurface and peripheral damage induced by the energetic ions in the underlying substrate. The in situ mitigation of subsurface damage induced by He(+)/Ne(+) ion exposures in silicon via a synchronized infrared pulsed laser-assisted process is demonstrated. The pulsed laser assist provides highly localized in situ photothermal energy which reduces the implantation and defect concentration by greater than 90%. The laser-assisted exposure process is also shown to reduce peripheral defects in He(+) patterned graphene, which makes this process an attractive candidate for direct-write patterning of 2D materials. These results offer a necessary solution for the applicability of high-resolution direct-write nanoscale material processing via focused ion beams. PMID:26864147

  20. Dynamics of neutrals and ions in an ultrafast laser produced Zn plasma

    SciTech Connect

    Smijesh, N.; Rao, Kavya H.; Philip, Reji

    2015-03-15

    Optical time of flight dynamics of neutrals and ions in an ultrafast laser produced zinc plasma generated by irradiating a solid zinc target using 100 fs laser pulses is investigated. An acceleration of ions is observed which arises from internal Coulomb forces acting between charged species in the plasma. Some of the fast ions recombine with electrons in the plasma and generate fast neutrals. Plasma plume imaging performed at various ambient pressures indicates adiabatic expansion at lower pressures and plume front deceleration at higher pressures: at lower pressures the plume front-time (R-t) plot displays a linear expansion, shock wave model fits to the data at 5 Torr and at higher pressures the data fits better to the drag model. Furthermore, around an intermediate pressure of 10 Torr, the R-t plot fits to the shock wave model at earlier stages of plasma expansion, while it fits to the drag model at the later stages. These investigations provide relevant information on the acceleration of ions and neutrals in an expanding zinc plasma plume produced by ultrafast laser pulses.

  1. In Situ Mitigation of Subsurface and Peripheral Focused Ion Beam Damage via Simultaneous Pulsed Laser Heating.

    PubMed

    Stanford, Michael G; Lewis, Brett B; Iberi, Vighter; Fowlkes, Jason D; Tan, Shida; Livengood, Rick; Rack, Philip D

    2016-04-01

    Focused helium and neon ion (He(+)/Ne(+)) beam processing has recently been used to push resolution limits of direct-write nanoscale synthesis. The ubiquitous insertion of focused He(+)/Ne(+) beams as the next-generation nanofabrication tool-of-choice is currently limited by deleterious subsurface and peripheral damage induced by the energetic ions in the underlying substrate. The in situ mitigation of subsurface damage induced by He(+)/Ne(+) ion exposures in silicon via a synchronized infrared pulsed laser-assisted process is demonstrated. The pulsed laser assist provides highly localized in situ photothermal energy which reduces the implantation and defect concentration by greater than 90%. The laser-assisted exposure process is also shown to reduce peripheral defects in He(+) patterned graphene, which makes this process an attractive candidate for direct-write patterning of 2D materials. These results offer a necessary solution for the applicability of high-resolution direct-write nanoscale material processing via focused ion beams.

  2. Tetravalent Chromium (Cr(4+)) as Laser-Active Ion for Tunable Solid-State Lasers

    NASA Technical Reports Server (NTRS)

    Seas, A.; Petricevic, V.; Alfano, Robert R.

    1993-01-01

    During 10/31/92 - 3/31/93, the following summarizes our major accomplishments: (1) the self-mode-locked operation of the Cr:forsterite laser was achieved; (2) synchronous pumping was used to mode lock the forsterite laser resulting in picosecond pulses, which in turn provided the starting mechanism for self-mode-locking; and (3) the pulses generated had a FWHW of 105 fs and were tunable between 1230 - 1270 nm.

  3. High power laser coupling to carbon nano-tubes and ion Coulomb explosion

    SciTech Connect

    K, Magesh Kumar K; Tripathi, V. K.

    2013-09-15

    Linear and non linear interaction of laser with an array of carbon nanotubes is investigated. The ac conductivity of nanotubes, due to uneven response of free electrons in them to axial and transverse fields, is a tensor. The propagation constant for p-polarization shows resonance at a specific frequency that varies with the direction of laser propagation. It also shows surface plasmon resonance at ω=ω{sub p}/√(2), where ω{sub p} is the plasma frequency of free electrons inside a nanotube, assumed to be uniform plasma cylinder. The attenuation constant is also resonantly enhanced around these frequencies. At large laser amplitude, the nanotubes behave as thin plasma rods. As the electrons get heated, the nanotubes undergo hydrodynamic expansion. At an instant when plasma frequency reaches ω{sub p}=√(2)ω, the electron temperature rises rapidly and then saturates. For a Gaussian laser beam, the heating rate is maximum on the laser axis and falls off with the distance r from the axis. When the excursion of the electrons Δ is comparable or larger than the radius of the nanotube r{sub c}, the nanotubes undergo ion Coulomb explosion. The distribution function of ions turns out to be a monotonically decreasing function of energy.

  4. High power laser coupling to carbon nano-tubes and ion Coulomb explosion

    NASA Astrophysics Data System (ADS)

    K, Magesh Kumar K.; Tripathi, V. K.

    2013-09-01

    Linear and non linear interaction of laser with an array of carbon nanotubes is investigated. The ac conductivity of nanotubes, due to uneven response of free electrons in them to axial and transverse fields, is a tensor. The propagation constant for p-polarization shows resonance at a specific frequency that varies with the direction of laser propagation. It also shows surface plasmon resonance at ω =ωp/√2 , where ωp is the plasma frequency of free electrons inside a nanotube, assumed to be uniform plasma cylinder. The attenuation constant is also resonantly enhanced around these frequencies. At large laser amplitude, the nanotubes behave as thin plasma rods. As the electrons get heated, the nanotubes undergo hydrodynamic expansion. At an instant when plasma frequency reaches ωp=√2 ω, the electron temperature rises rapidly and then saturates. For a Gaussian laser beam, the heating rate is maximum on the laser axis and falls off with the distance r from the axis. When the excursion of the electrons Δ is comparable or larger than the radius of the nanotube rc, the nanotubes undergo ion Coulomb explosion. The distribution function of ions turns out to be a monotonically decreasing function of energy.

  5. The electron-ion dynamics in ionization of lithium carbide molecule under femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaoqin; Wang, Feng; Hong, Xuhai; Su, Wenyong; Gou, Bingcong; Chen, Huimin

    2016-08-01

    The electron-ion dynamics of the linear lithium carbide molecule under femtosecond laser pulses have been investigated in the framework of Ehrenfest molecular dynamics, in which valence electrons are treated quantum mechanically by time-dependent density functional theory (TDDFT) and ions are described classically. The on- and off-resonant multiphoton ionization processes have been induced by regulating laser frequency and laser intensity. The laser pulse with on-resonant frequency induces pronounced enhancement in electron ionization, bond length vibration, and energy absorption. Moreover, the coulomb explosion is preferred to occur in the on-resonant case, which is in qualitative agreement with previous theoretical investigations. The subtle relations between escaped electron number and absorbed photon number are well discussed with the increasing of laser intensity. Finally, the effect of self-interaction error is analyzed by comparing escaped electron number calculated with LDA and LDA-ADSIC. And the revTPSS-meta-GGA, a currently more accurate nonempirical exchange-correlation energy functional from a point of static density functional theory, is introduced to display its capability for the description of ionization process within nonlinear and the nonperturbative regime of isolated systems.

  6. High efficiency picosecond pulse generation in the 675-930 nm region from a dye laser synchronously pumped by an argon-ion laser. Technical report

    SciTech Connect

    Bado, P.; Dupuy, C.; Wilson, K.R.; Boggy, R.; Bowen, J.

    1983-04-01

    Picosecond pulses tunable from 675 to 930 micrometers have been obtained from a dye-laser synchronously pumped at 514.5 micrometers by a mode-locked Argon-ion laser. Peak energy conversion efficiencies between 10% and 29% are observed with pulse durations between 1.7 ps and 16 ps as measured by autocorrelation.

  7. Efficient generation of fast ions from surface modulated nanostructure targets irradiated by high intensity short-pulse lasers

    SciTech Connect

    Andreev, Alexander; Kumar, Naveen; Pukhov, Alexander; Platonov, Konstantin

    2011-10-15

    It's shown that the imposition of sub-laser wavelength relief structures on the surface of mass-limited-targets results into several folds higher short-pulse laser absorption, and consequently the efficient generation of fast ions. The optimum relief parameters for enhanced short-pulse laser absorption and higher ion acceleration are estimated numerically by particle-in-cell simulations and then corroborated by analytical scalings. The stability of the pre-imposed surface modulation during the laser pulse foil interaction is also examined.

  8. Laser photodetachment diagnostics of a 1/3-size negative hydrogen ion source for NBI

    SciTech Connect

    Geng, S.; Tsumori, K.; Nakano, H.; Kisaki, M.; Ikeda, K.; Takeiri, Y.; Osakabe, M.; Nagaoka, K.; Kaneko, O.

    2015-04-08

    To investigate the flows of charged particles in front of the plasma grid (PG) in a negative hydrogen ion source, the information of the local densities of electrons and negative hydrogen ions (H-) are necessary. For this purpose, the laser photodetachment is applied for pure hydrogen plasmas and Cs-seeded plasma in a 1/3-size negative hydrogen ion source in NIFS-NBI test stand. The H- density obtained by photodetachment is calibrated by the results from cavity ring-down (CRD). The pressure dependence and PG bias dependence of the local H- density are presented and discussed. The results show that H- density increases significantly by seeding Cs into the plasma. In Cs-seeded plasma, relativity exists between the H- ion density and plasma potential.

  9. Laser damage resistance of hafnia thin films deposited by electron beam deposition, reactive low voltage ion plating, and dual ion beam sputtering

    SciTech Connect

    Gallais, Laurent; Capoulade, Jeremie; Natoli, Jean-Yves; Commandre, Mireille; Cathelinaud, Michel; Koc, Cian; Lequime, Michel

    2008-05-01

    A comparative study is made of the laser damage resistance of hafnia coatings deposited on fused silica substrates with different technologies: electron beam deposition (from Hf or HfO2 starting material), reactive low voltage ion plating, and dual ion beam sputtering.The laser damage thresholds of these coatings are determined at 1064 and 355 nm using a nanosecond pulsed YAG laser and a one-on-one test procedure. The results are associated with a complete characterization of the samples: refractive index n measured by spectrophotometry, extinction coefficient k measured by photothermal deflection, and roughness measured by atomic force microscopy.

  10. High-power Ti:sapphire lasers for spectroscopy of antiprotonic atoms and radioactive ions

    NASA Astrophysics Data System (ADS)

    Hori, M.; Dax, A.; Soter, A.

    The ASACUSA collaboration has developed injection-seeded Ti:sapphire lasers of linewidth Γpl ˜ 6 MHz, pulse energy 50-100 mJ, and output wavelength λ = 726-941 nm. They are being used in two-photon spectroscopy experiments of antiprotonic helium atoms at the Antiproton Decelerator (AD) of CERN. Ti:sapphire lasers of larger linewidth Γpl ˜ 100 MHz but more robust design will also be used in collinear resonance ionization spectroscopy (CRIS) experiments of neutron-deficient francium ions at the ISOLDE facility.

  11. High-power Ti:sapphire lasers for spectroscopy of antiprotonic atoms and radioactive ions

    NASA Astrophysics Data System (ADS)

    Hori, M.; Dax, A.; Soter, A.

    2012-12-01

    The ASACUSA collaboration has developed injection-seeded Ti:sapphire lasers of linewidth Γpl ˜ 6 MHz, pulse energy 50-100 mJ, and output wavelength λ = 726-941 nm. They are being used in two-photon spectroscopy experiments of antiprotonic helium atoms at the Antiproton Decelerator (AD) of CERN. Ti:sapphire lasers of larger linewidth Γpl ˜ 100 MHz but more robust design will also be used in collinear resonance ionization spectroscopy (CRIS) experiments of neutron-deficient francium ions at the ISOLDE facility.

  12. Effect of citrate ions on laser ablation of Ag foil in aqueous medium

    NASA Astrophysics Data System (ADS)

    Sisková, K.; Vlcková, B.; Turpin, P.-Y.; Fayet, C.; Hromádková, J.; Slouf, M.

    2007-04-01

    Promoting effect of citrate in 1 × 10-5-1×10-2 M concentrations on laser ablation (LA) of a Ag foil in aqueous solution performed by ns laser pulses at 1064 nm is reported. Furthermore, adsorption of citrate ions was found to increase markedly the stability of the resulting LA-Ag hydrosol. The results are discussed on the basis of comparison of surface plasmon extinction spectral characteristics, transmission electron microscopy images, nanoparticle size distributions and surface-enhanced Raman scattering (SERS) spectral tests of hydrosols resulting from LA in neutral and acidic aqueous citrate solutions and in pure water.

  13. Device for simultaneous multiple-line mode locking of an argon-ion laser

    SciTech Connect

    Kitahara, T.

    1987-11-01

    An acousto-optic device that can simultaneously mode lock multiple lines of a laser source has been designed and demonstrated. The device is an intracavity acousto-optic modulator with an end mirror. Multiple argon-ion laser lines at 476.5, 488.0, 496.5, and 514.5 nm were simultaneously modulated by using this device. Pulse trains with pulses having a width of approximately 100 psec FWHM at a repetition of 130 MHz were obtained for each line.

  14. Direct evidence of strongly inhomogeneous energy deposition in target heating with laser-produced ion beams.

    PubMed

    Brambrink, E; Schlegel, T; Malka, G; Amthor, K U; Aléonard, M M; Claverie, G; Gerbaux, M; Gobet, F; Hannachi, F; Méot, V; Morel, P; Nicolai, P; Scheurer, J N; Tarisien, M; Tikhonchuk, V; Audebert, P

    2007-06-01

    We report on strong nonuniformities in target heating with intense, laser-produced proton beams. The observed inhomogeneity in energy deposition can strongly perturb equation of state (EOS) measurements with laser-accelerated ions which are planned in several laboratories. Interferometric measurements of the target expansion show different expansion velocities on the front and rear surfaces, indicating a strong difference in local temperature. The nonuniformity indicates at an additional heating mechanism, which seems to originate from electrons in the keV range. PMID:17677318

  15. Dynamics of ions produced by laser ablation of several metals at 193 nm

    SciTech Connect

    Baraldi, G.; Perea, A.; Afonso, C. N.

    2011-02-15

    This work reports the study of ion dynamics produced by ablation of Al, Cu, Ag, Au, and Bi targets using nanosecond laser pulses at 193 nm as a function of the laser fluence from threshold up to 15 J cm{sup -2}. An electrical (Langmuir) probe has been used for determining the ion yield as well as kinetic energy distributions. The results clearly evidence that ablation of Al shows unique features when compared to other metals. The ion yield both at threshold (except for Al, which shows a two-threshold-like behavior) and for a fixed fluence above threshold scale approximately with melting temperature of the metal. Comparison of the magnitude of the yield reported in literature using other wavelengths allows us to conclude its dependence with wavelength is not significant. The evolution of the ion yield with fluence becomes slower for fluences above 4-5 J cm{sup -2} with no indication of saturation suggesting that ionization processes in the plasma are still active up to 15 J cm{sup -2} and production of multiple-charged ions are promoted. This dependence is mirrored in the proportion of ions with kinetic energies higher than 200 eV. This proportion is not significant around threshold fluence for all metals except for Al, which is already 20%. The unique features of Al are discussed in terms of the energy of laser photons (6.4 eV) that is enough to induce direct photoionization from the ground state only in the case of this metal.

  16. Modifications in surface, structural and mechanical properties of brass using laser induced Ni plasma as an ion source

    NASA Astrophysics Data System (ADS)

    Ahmad, Shahbaz; Bashir, Shazia; Rafique, M. Shahid; Yousaf, Daniel

    2016-03-01

    Laser induced Ni plasma has been employed as source of ion implantation for surface, structural and mechanical properties of brass. Excimer laser (248 nm, 20 ns, 120mJ and 30 Hz) was used for the generation of Ni plasma. Thomson parabola technique was employed to estimate the energy of generated ions using CR39 as a detector. In response to stepwise increase in number of laser pulses from 3000 to 12000, the ion dose varies from 60 × 1013 to 84 × 1016 ions/cm2 with constant energy of 138 KeV. SEM analysis reveals the growth of nano/micro sized cavities, pores, pits, voids and cracks for the ion dose ranging from 60 × 1013 to 70 × 1015 ions/cm2. However, at maximum ion dose of 84 × 1016 ions/cm2 the granular morphology is observed. XRD analysis reveals that new phase of CuZnNi (200) is formed in the brass substrate after ion implantation. However, an anomalous trend in peak intensity, crystallite size, dislocation line density and induced stresses is observed in response to the implantation with various doses. The increase in ion dose causes to decrease the Yield Stress (YS), Ultimate Tensile Strength (UTS) and hardness. However, for the maximum ion dose the highest values of these mechanical properties are achieved. The variations in the mechanical properties are correlated with surface and crystallographical changes of ion implanted brass.

  17. Improving beam spectral and spatial quality by double-foil target in laser ion acceleration for ion-driven fast ignition

    NASA Astrophysics Data System (ADS)

    Huang, Chengkun

    2010-11-01

    Mid-Z ion driven fast ignition inertial fusion [1] requires ion beams of 100s of MeV energy and < 10% energy spread. An overdense nm-scale foil target driven by a high intensity laser pulse can produce an ion beam that has attractive properties for this application. The Break Out Afterburner (BOA) [2] is one laser-ion acceleration mechanism proposed to generate such beams, however the late stages of the BOA tend to produce too large of an energy spread. The spectral and spatial qualities of the beam quickly evolve as the ion beam and co-moving electrons continue to interact with the laser. Here we show how use of a second target foil placed behind a nm-scale foil can substantially reduce the temperature of the co-moving electrons and improve the ion beam energy spread [3]. Particle-In-Cell simulations reveal the dynamics of the ion beam under control. Optimal conditions for improving the spectral and spatial spread of the ion beam is explored for current laser and target parameters, leading to generation of ion beams of energy 100s of MeV and 6% energy spread, a vital step for realizing ion-driven fast ignition. [4pt] [1] M. Roth et al., Phys. Rev. Lett. 86, 436 (2001); M. Temporal, J. J. Honrubia, and S. Atzeni, Phys. of Plasmas 9, 3098 (2002). [2] L. Yin, B. J. Albright, B. M. Hegelich, and J. C. Fern'andez, Laser and Part. Beams 24, 291 (2006). [3] C.-K. Huang, B. J. Albright, L. Yin, H.-C. Wu et al., submitted to Phys. Rev. Lett.

  18. Experiment and modeling of laser photodetachment of negative ions in helium oxygen barrier discharges

    NASA Astrophysics Data System (ADS)

    Tschiersch, Robert; Nemschokmichal, Sebastian; Meichsner, Jürgen

    2015-09-01

    Helium oxygen discharges operating at atmospheric pressure are of great interest for applications, such as surface treatment of biological samples. Helium as the buffer gas keeps the driving power low, and oxygen serves as the source of radicals. The large electronegativity of oxygen results in the formation of negative ions which in turn have a remarkable influence on the discharge development. To point out this role of negative ions, the change of the discharge behavior after the laser photodetachment of negative ions is measured in a helium oxygen barrier discharge. These measurements reveal a lower breakdown voltage when firing the laser during the pre-phase of the discharge. The reason is the additional pre-ionization by the detached electrons which was proved by an 1D numeric fluid modeling. The next step is the determination of absolute number densities of negative ions by a comparison of the experimental parameter variations with those from the modeling. Furthermore, the actual role of negative ions on the discharge behavior will be emphasized by the modeling.

  19. Low-temperature, site selective graphitization of SiC via ion implantation and pulsed laser annealing

    SciTech Connect

    Lemaitre, Maxime G.; Tongay, Sefaattin; Wang, Xiaotie; Venkatachalam, Dinesh K.; Elliman, Robert G.; Fridmann, Joel; Gila, Brent P.; Appleton, Bill R.; Hebard, Arthur F.; Ren, Fan

    2012-05-07

    A technique is presented to selectively graphitize regions of SiC by ion implantation and pulsed laser annealing (PLA). Nanoscale features are patterned over large areas by multi-ion beam lithography and subsequently converted to few-layer graphene via PLA in air. Graphitization occurs only where ions have been implanted and without elevating the temperature of the surrounding substrate. Samples were characterized using Raman spectroscopy, ion scattering/channeling, SEM, and AFM, from which the degree of graphitization was determined to vary with implantation species, damage and dose, laser fluence, and pulsing. Contrasting growth regimes and graphitization mechanisms during PLA are discussed.

  20. Passive Q-switching of diode-pumped Yb:YAG microchip laser with ion-implanted GaAs

    NASA Astrophysics Data System (ADS)

    Wang, Yonggang; Ma, Xiaoyu; Zhong, Bin; Wang, Desong; Zhang, Qiulin; Feng, Baohua

    2004-01-01

    We reported a passive Q-switched diode laser pumped Yb:YAG microchip laser with an ion-implanted semi-insulating GaAs wafer. The wafer was implanted with 400-keV As^(+) in the concentration of 10^(16) ions/cm^(2). To decrease the non-saturable loss, we annealed the ion-implanted GaAs at 500 oC for 5 minutes and coated both sides of the ion-implanted GaAs with antireflection (AR) and highreflection (HR) films, respectively. Using GaAs wafer as an absorber and an output coupler, we obtained 52-ns pulse duration of single pulse.

  1. Transverse characteristics of short-pulse laser-produced ion beams: a study of the acceleration dynamics.

    PubMed

    Brambrink, E; Schreiber, J; Schlegel, T; Audebert, P; Cobble, J; Fuchs, J; Hegelich, M; Roth, M

    2006-04-21

    We report on first measurements of the transverse characteristics of laser-produced energetic ion beams in direct comparison to results for laser accelerated proton beams. The experiments show the same low emittance for ion beams as already found for protons. Additionally, we demonstrate that the divergence is influenced by the charge over mass ratio of the accelerated species. From these observations we deduced scaling laws for the divergence of ions as well as the temporal evolution of the ion source size. PMID:16712164

  2. The generation, detection and measurement of laser-induced carbon plasma ions and their implantation effects on brass substrate

    NASA Astrophysics Data System (ADS)

    Ahmad, Shahbaz; Bashir, Shazia; Shahid Rafique, M.; Yousaf, Daniel; Ahmad, Riaz

    2016-05-01

    The generation, detection and measurement of laser-induced carbon plasma ions and their implantation effects on brass substrate have been investigated. Thomson parabola technique was employed to measure the energy and flux of carbon ions. The magnetic field of strength 80 mT was applied on the graphite plasma plume to provide an appropriate trajectory to the generated ions. The energy of carbon ions is 678 KeV for laser fluence of 5.1 J/cm2 which was kept constant for all exposures. The flux of ions varies from 32 × 1011 to 72 × 1014 ions/cm2 for varying numbers of laser pulses from 3000 to 12,000. In order to explore the ion irradiation effects on brass, four brass substrates were irradiated by carbon ions of different flux. Scanning electron microscope (SEM) and X-ray diffractometer (XRD) are used to analyze the surface morphology and crystallographic structure of ion-implanted brass, respectively. SEM analysis reveals the formation and growth of nano-/micro-sized cavities, pores and pits for the various ion flux for varying numbers of laser pulses from 3000 to 12,000. By increasing ion flux by increasing the number of pulses up to 9000 shots, the dendritic structures initiate to grow along with cavities and pores. At the maximum ion flux for 12,000 shots, the unequiaxed dendritic structures become distinct and the distance between the dendrites is decreased, whereas cavities, pores and pits are completely finished. The XRD analysis reveals that a new phase of ZnC (0012) is formed in the brass substrate after ion implantation. Universal tensile testing machine and Vickers microhardness tester are used to explore the yield stress, ultimate tensile strength and microhardness of ion-implanted brass substrate. The mechanical properties monotonically increase by increasing the ion flux. Variations in mechanical properties are correlated with surface and structural modifications of brass.

  3. Ion-neutral chemistry at ultralow energies: dynamics of reactive collisions between laser-cooled Ca+ ions and Rb atoms in an ion-atom hybrid trap†

    NASA Astrophysics Data System (ADS)

    Hall, Felix H. J.; Eberle, Pascal; Hegi, Gregor; Raoult, Maurice; Aymar, Mireille; Dulieu, Olivier; Willitsch, Stefan

    2013-08-01

    Cold chemical reactions between laser-cooled Ca+ ions and Rb atoms were studied in an ion-atom hybrid trap. Reaction rate constants were determined in the range of collision energies ⟨E coll⟩/k B=20 mK-20 K. The lowest energies were achieved in experiments using single localised Ca+ ions. Product branching ratios were studied using resonant-excitation mass spectrometry. The dynamics of the reactive processes in this system (non-radiative and radiative charge transfer as well as radiative association leading to the formation of CaRb+ molecular ions) have been analysed using high-level quantum-chemical calculations of the potential energy curves of CaRb+ and quantum-scattering calculations for the radiative channels. For the present low-energy scattering experiments, it is shown that the energy dependence of the reaction rate constants is governed by long-range interactions in line with the classical Langevin model, but their magnitude is determined by short-range non-adiabatic and radiative couplings which only weakly depend on the asymptotic energy. The quantum character of the collisions is predicted to manifest itself in the occurrence of narrow shape resonances at well-defined collision energies. The present results highlight both universal and system-specific phenomena in cold ion-neutral reactive collisions.

  4. Application of laser produced ion beams to nuclear analysis of materials

    NASA Astrophysics Data System (ADS)

    Mima, Kunioki; Fujita, K.; Azuma, H.; Yamazaki, A.; Kato, Y.; Okuda, C.; Ukyo, Y.; Sawada, H.; Gonzalez-Arrabal, Raquel; Perlado, J. M.; Nishimura, H.; Nakai, S.

    2013-11-01

    The ion beam driven nuclear analysis has been developed for many years by using various electrostatic accelerators. A proton micro-beam with the beam diameter of ˜1.5 μm at Takasaki Ion Acceleration for Advanced Radiation Application (TIARA), JAEA was used to analyze the positive electrode of the Li-ion battery with PIGE and PIXE. WThe PIGE and PIXE images of Li and Ni respectively for LixNi0.8Co0.15Al0.05O2(x = 0.75 ˜ 1.0) anodes have been taken. The PIGE images of LixNi0.8Co0.15Al0.05O2 particles and the depth profile of the Li density have been obtained with high spatial resolution (a few μm). The images of the Li density distribution are very useful for the R&D of the Li ion battery. In order to make the in-situ ion beam analysis of the Li battery possible, a compact accelerator for a high quality MeV proton beam is necessary. Form this point of view, the diagnostics of Li ion battery is an appropriate field for the applications of laser produced ion beams.

  5. Review on developments in LIS (laser ion source) at the IPPLM and its possible applications in photonics

    NASA Astrophysics Data System (ADS)

    Gasior, P.; Rosinski, M.

    2013-10-01

    One of the techniques which had the biggest impact on the development of microelectronics, optoelectronics, photonics and other similar technologies was doping the substrates with various elements. Although many techniques have been developed resulting in reliable industrial designs, still there is a need of further development and optimization of some of them for specific applications. A very interesting method of doping is the ion implantation based on LIS (Laser Ion Source). The great advantage of this method is its ability to implant ions from any solid state material onto any substrate. Besides - a control of the laser irradiation parameters gives also a flexibility in the parameters of the implantation process, i.e. the ion energy which corresponds to the implantation depth and the ion flux which results in the concentration. On the other hand there are also drawbacks of the direct method - usually the power density of the laser beam needs to be higher than that offered by standard industrial solution and together with the dopant the contaminations present in the projectile are implanted. Another issue for the applications requiring high precision of the implanted layer depth and width is the relatively broad energy spread of the laser produced ions. To deal with this problems the research at the IPPLM was focused on the extent characterization of laser produced ion streams in the direct variant of the method and optimization of the method with the application of electrostatic field to accelerate, focus and shape the ion beams.

  6. Electron-ion and ion-ion potentials for modeling warm dense matter: Applications to laser-heated or shock-compressed Al and Si

    NASA Astrophysics Data System (ADS)

    Dharma-wardana, M. W. C.

    2012-09-01

    The pair interactions Uij(r) determine the thermodynamics and linear transport properties of matter via the pair-distribution functions (PDFs), i.e., gij(r). Great simplicity is achieved if Uij(r) could be directly used to predict material properties via classical simulations, avoiding many-body wave functions. Warm dense matter (WDM) is encountered in quasiequilibria where the electron temperature Te differs from the ion temperature Ti, as in laser-heated or in shock-compressed matter. The electron PDFs gee(r) as perturbed by the ions are used to evaluate fully nonlocal exchange-correlation corrections to the free energy, using hydrogen as an example. Electron-ion potentials for ions with a bound core are discussed with Al and Si as examples, for WDM with Te≠Ti, and valid for times shorter than the electron-ion relaxation time. In some cases the potentials develop attractive regions and then become repulsive and “Yukawa-like” for higher Te. These results clarify the origin of initial phonon hardening and rapid release. Pair potentials for shock-heated WDM show that phonon hardening would not occur in most such systems. Defining meaningful quasiequilibrium static transport coefficients consistent with the dynamic values is addressed. There seems to be no meaningful “static conductivity” obtainable by extrapolating experimental or theoretical σ(ω,Ti,Te) to ω→0, unless Ti→Te as well. Illustrative calculations of quasistatic resistivities R(Ti,Te) of laser-heated as well as shock-heated aluminum and silicon are presented using our pseudopotentials, pair potentials, and classical integral equations. The quasistatic resistivities display clear differences in their temperature evolutions, but are not the strict ω→0 limits of the dynamic values.

  7. Electron-ion and ion-ion potentials for modeling warm dense matter: Applications to laser-heated or shock-compressed Al and Si.

    PubMed

    Dharma-wardana, M W C

    2012-09-01

    The pair interactions Uij(r) determine the thermodynamics and linear transport properties of matter via the pair-distribution functions (PDFs), i.e., gij(r). Great simplicity is achieved if Uij(r) could be directly used to predict material properties via classical simulations, avoiding many-body wave functions. Warm dense matter (WDM) is encountered in quasiequilibria where the electron temperature Te differs from the ion temperature Ti, as in laser-heated or in shock-compressed matter. The electron PDFs gee(r) as perturbed by the ions are used to evaluate fully nonlocal exchange-correlation corrections to the free energy, using hydrogen as an example. Electron-ion potentials for ions with a bound core are discussed with Al and Si as examples, for WDM with Te≠Ti, and valid for times shorter than the electron-ion relaxation time. In some cases the potentials develop attractive regions and then become repulsive and "Yukawa-like" for higher Te. These results clarify the origin of initial phonon hardening and rapid release. Pair potentials for shock-heated WDM show that phonon hardening would not occur in most such systems. Defining meaningful quasiequilibrium static transport coefficients consistent with the dynamic values is addressed. There seems to be no meaningful "static conductivity" obtainable by extrapolating experimental or theoretical σ(ω,Ti,Te) to ω→0, unless Ti→Te as well. Illustrative calculations of quasistatic resistivities R(Ti,Te) of laser-heated as well as shock-heated aluminum and silicon are presented using our pseudopotentials, pair potentials, and classical integral equations. The quasistatic resistivities display clear differences in their temperature evolutions, but are not the strict ω→0 limits of the dynamic values.

  8. Optical shaping of gas targets for laser-plasma ion sources

    NASA Astrophysics Data System (ADS)

    Dover, N. P.; Cook, N.; Tresca, O.; Ettlinger, O.; Maharjan, C.; Polyanskiy, M. N.; Shkolnikov, P.; Pogorelsky, I.; Najmudin, Z.

    2016-02-01

    We report on the experimental demonstration of a technique to generate steep density gradients in gas-jet targets of interest to laser-plasma ion acceleration. By using an intentional low-energy prepulse, we generated a hydrodynamic blast wave in the gas to shape the target prior to the arrival of an intense CO2 λ≈ 10m drive pulse. This technique has been recently shown to facilitate the generation of ion beams by shockwave acceleration (Tresca et al., Phys. Rev. Lett., vol. 115 (9), 2015, 094802). Here, we discuss and introduce a model to understand the generation of these blast waves and discuss in depth the experimental realisation of the technique, supported by hydrodynamics simulations. With appropriate prepulse energy and timing, this blast wave can generate steepened density gradients as short as &ap 20μm (1/e), opening up new possibilities for laser-plasma studies with near-critical gaseous targets.

  9. Process for ion-assisted laser deposition of biaxially textured layer on substrate

    DOEpatents

    Russo, Richard E.; Reade, Ronald P.; Garrison, Stephen M.; Berdahl, Paul

    1995-01-01

    A process for depositing a biaxially aligned intermediate layer over a non-single crystal substrate is disclosed which permits the subsequent deposition thereon of a biaxially oriented superconducting film. The process comprises depositing on a substrate by laser ablation a material capable of being biaxially oriented and also capable of inhibiting the migration of substrate materials through the intermediate layer into such a superconducting film, while simultaneously bombarding the substrate with an ion beam. In a preferred embodiment, the deposition is carried out in the same chamber used to subsequently deposit a superconducting film over the intermediate layer. In a further aspect of the invention, the deposition of the superconducting layer over the biaxially oriented intermediate layer is also carried out by laser ablation with optional additional bombardment of the coated substrate with an ion beam during the deposition of the superconducting film.

  10. Process for ion-assisted laser deposition of biaxially textured layer on substrate

    DOEpatents

    Russo, R.E.; Reade, R.P.; Garrison, S.M.; Berdahl, P.

    1995-07-11

    A process for depositing a biaxially aligned intermediate layer over a non-single crystal substrate is disclosed which permits the subsequent deposition thereon of a biaxially oriented superconducting film. The process comprises depositing on a substrate by laser ablation a material capable of being biaxially oriented and also capable of inhibiting the migration of substrate materials through the intermediate layer into such a superconducting film, while simultaneously bombarding the substrate with an ion beam. In a preferred embodiment, the deposition is carried out in the same chamber used to subsequently deposit a superconducting film over the intermediate layer. In a further aspect of the invention, the deposition of the superconducting layer over the biaxially oriented intermediate layer is also carried out by laser ablation with optional additional bombardment of the coated substrate with an ion beam during the deposition of the superconducting film. 8 figs.

  11. Negative ions: The overlooked species in thin film growth by pulsed laser deposition

    SciTech Connect

    Esposito, M.; Bator, M.; Lippert, T.; Schneider, C. W.; Wokaun, A.; Doebeli, M.

    2011-11-07

    Plasma plume species from a ceramic La{sub 0.4}Ca{sub 0.6}MnO{sub 3} target were studied by plasma mass spectrometry as a function of laser fluence, background gas, and deposition pressure to understand the interplay between plasma composition and oxide thin film growth by pulsed laser deposition. The plume composition reveals a significant contribution of up to 24% of negative ions, most notably using a N{sub 2}O background. The significance of negative ions for thin film growth is shown for La{sub 0.4}Ca{sub 0.6}MnO{sub 3} films grown in different background conditions where the best structural properties coincide with the largest amount of negative plasma species.

  12. Focusing dynamics of high-energy density, laser-driven ion beams.

    PubMed

    Chen, S N; d'Humières, E; Lefebvre, E; Romagnani, L; Toncian, T; Antici, P; Audebert, P; Brambrink, E; Cecchetti, C A; Kudyakov, T; Pipahl, A; Sentoku, Y; Borghesi, M; Willi, O; Fuchs, J

    2012-02-01

    The dynamics of the focusing of laser-driven ion beams produced from concave solid targets was studied. Most of the ion beam energy is observed to converge at the center of the cylindrical targets with a spot diameter of 30  μm, which can be very beneficial for applications requiring high beam energy densities. Also, unbalanced laser irradiation does not compromise the focusability of the beam. However, significant filamentation occurs during the focusing, potentially limiting the localization of the energy deposition region by these beams at focus. These effects could impact the applicability of such high-energy density beams for applications, e.g., in proton-driven fast ignition. PMID:22400936

  13. Collisionless shocks driven by 800 nm laser pulses generate high-energy carbon ions

    SciTech Connect

    Zhang, H.; Shen, B. F. Wang, W. P.; Xu, Y.; Liu, Y. Q.; Liang, X. Y.; Leng, Y. X.; Li, R. X. Xu, Z. Z.; Yan, X. Q.; Chen, J. E.

    2015-01-15

    We present experimental studies on ion acceleration from diamond-like carbon (DLC) foils irradiated by 800 nm, linearly polarized laser pulses with peak intensity of 1.7 × 10{sup 19 }W/cm{sup 2} to 3.5 × 10{sup 19 }W/cm{sup 2} at oblique incidence. Diamond-like carbon foils are heated by the prepulse of a high-contrast laser pulse and expand to form plasmas of near-critical density caused by thermal effect before the arrival of the main pulse. It is demonstrated that carbon ions are accelerated by a collisionless shock wave in slightly overdense plasma excited by forward-moving hot electrons generated by the main pulse.

  14. Tetravalent chromium (Cr(4+)) as laser-active ion for tunable solid-state lasers

    NASA Technical Reports Server (NTRS)

    Seas, A.; Petricevic, V.; Alfano, Robert R.

    1993-01-01

    Major accomplishments under NASA grant NAG-1-1346 are summarized. (1) numerical modeling of the four mirror astigmatically compensated, Z-fold cavity was performed and several design parameters to be used for the construction of a femtosecond forsterite laser were revealed by simulation. (2) femtosecond pulses from a continuous wave mode-locked chromium doped forsterite laser were generated. The forsterite laser was actively mode-locked using an acousto-optic modulator operating at 78 MHz with two Brewster high dispersion glass prisms for intra-cavity chirp compensation. Transform-limited sub-100-fs pulses were routinely generated in the TEM(sub 00) mode with 85 mW of continuous power tunable over 1230-1280 nm. The shortest pulses of 60-fs pulsewidth were measured. (3) Self-mode-locked operation of the Cr:forsterite laser was achieved. Synchronous pumping was used to mode lock the forsterite laser resulting in picosecond pulses, which in turn provided the starting mechanism for self-mode-locking. The pulses generated had an FWHM of 105 fs and were tunable between 1230-1270 nm. (4) Numerical calculations indicated that the pair of SF 14 prisms used in the cavity compensated for quadratic phase but introduced a large cubic phase term. Further calculations of other optical glasses indicated that a pair of SFN 64 prisms can introduce the same amount of quadratic phase as SF 14 prisms but introduce a smaller cubic phase. When the SF 14 prisms were replaced by SFN 64 prisms the pulsewidth was reduced to 50 fs. Great improvement was observed in the stability of the self mode-locked forsterite laser and in the ease of achieving mode locking. Using the same experimental arrangement and a new forsterite crystal with improved FOM the pulse width was reduced to 36 fs.

  15. Laser Ion Acceleration from the Interaction of Ultra-Intense laser Pulse with thi foils

    SciTech Connect

    Allen, M

    2004-03-12

    The discovery that ultra-intense laser pulses (I > 10{sup 18} W/cm{sup 2}) can produce short pulse, high energy proton beams has renewed interest in the fundamental mechanisms that govern particle acceleration from laser-solid interactions. Experiments have shown that protons present as hydrocarbon contaminants on laser targets can be accelerated up to energies > 50 MeV. Different theoretical models that explain the observed results have been proposed. One model describes a front-surface acceleration mechanism based on the ponderomotive potential of the laser pulse. At high intensities (I > 10{sup 18} W/cm{sup 2}), the quiver energy of an electron oscillating in the electric field of the laser pulse exceeds the electron rest mass, requiring the consideration of relativistic effects. The relativistically correct ponderomotive potential is given by U{sub p} = ([1 + I{lambda}{sup 2}/1.3 x 10{sup 18}]{sup 1/2} - 1) m{sub o}c{sup 2}, where I{lambda}{sup 2} is the irradiance in W{micro}m{sup 2}/cm{sup 2} and m{sub o}c{sup 2} is the electron rest mass.At laser irradiance of I{lambda}{sup 2} {approx} 10{sup 20} W{micro}m{sup 2}/cm{sup 2}, the ponderomotive potential can be of order several MeV. A few recent experiments--discussed in Chapter 3 of this thesis--consider this ponderomotive potential sufficiently strong to accelerate protons from the front surface of the target to energies up to tens of MeV. Another model, known as Target Normal Sheath Acceleration (TNSA), describes the mechanism as an electrostatic sheath on the back surface of the laser target. According to the TNSA model, relativistic hot electrons created at the laser-solid interaction penetrate the foil where a few escape to infinity. The remaining hot electrons are retained by the target potential and establish an electrostatic sheath on the back surface of the target.

  16. Tetravalent chromium (Cr(4+)) as laser-active ion for tunable solid-state lasers

    NASA Technical Reports Server (NTRS)

    Seas, A.; Petricevic, V.; Alfano, Robert R.

    1992-01-01

    Generation of femtosecond pulses from a continuous-wave mode-locked chromium-doped forsterite (Cr(4+):Mg2SiO4) laser has been accomplished. The forsterite laser was actively mode-locked using an acousto-optic modulator operating at 78 MHz with two Brewster high-dispersion glass prisms for intra-cavity chirp compensation. Transform-limited sub-100-fs pulses were routinely generated in the TEM(sub 00) mode with 85 mW of continuous power (with 1 percent output coupler), tunable over 1230-1280 nm. The shortest pulses of 60-fs pulsewidth were measured.

  17. Fast ion acceleration from thin foils irradiated by ultra-high intensity, ultra-high contrast laser pulses

    SciTech Connect

    Prasad, R.; Ter-Avetisyan, S.; Doria, D.; Quinn, K. E.; Romagnani, L.; Zepf, M.; Borghesi, M.; Andreev, A. A.; Brenner, C. M.; Gallegos, P.; Carroll, D. C.; McKenna, P.; Tresca, O.; Dover, N. P.; Najmudin, Z.; Palmer, C. A. J.; Neely, D.; Green, J. S.; Foster, P. S.; Schreiber, J.; and others

    2011-09-19

    Ion acceleration resulting from the interaction of ultra-high intensity (2 x 10{sup 20 }W/cm{sup 2}) and ultra-high contrast ({approx}10{sup 10}) laser pulses with 0.05-10 {mu}m thick Al foils at normal (0 deg.) and 35 deg. laser incidence is investigated. When decreasing the target thickness from 10 {mu}m down to 0.05 {mu}m, the accelerated ions become less divergent and the ion flux increases, particularly at normal (0 deg.) laser incidence on the target. A laser energy conversion into protons of {approx}6.5% is estimated at 35 deg. laser incidence. Experimental results are in reasonable agreement with theoretical estimates and can be a benchmark for further theoretical and computational work.

  18. Acceleration of Ultra-Low Emittance Proton and Ion Beams with High Intensity Lasers

    NASA Astrophysics Data System (ADS)

    Cowan, Thomas E.

    2002-11-01

    Intense beams of several MeV protons and ions, generated by the interaction of high-intensity short pulse lasers with thin foils, have been observed by many researchers in recent years.(S.P. Hatchett et al., Phys. Plasmas 7, 2076 (2000); T.E. Cowan et al., Nucl. Inst. Meth. A 455, 130 (2000); R.A. Snavely et al., Phys. Rev. Lett. 85, 2945 (2000); S.C. Wilks et al., Phys. Plasmas 8, 532 (2000); E. Clark et al., Phys. Rev. Lett. 84, 670 (2000).) In experiments performed at the 100 TW LULI laser, we have succeeded to control the ion acceleration process to produce ultra high quality proton beams, whose transverse emittance is <0.006 π mm-mrad (rms-normalized), a factor of 100 lower than is typical of conventional RF linear accelerators. Within the envelope of the entire beam, we could focus individual proton beamlets to 100 nm spatial scales. This required control of the laser-plasma interaction, of the transport of MA currents of relativistic electrons through the target substrate, and of the surface topology and source material layering on the target foil rear-surface.(M. Roth et al., Phys. Rev. ST Accel. Beams 5, 061002 (2002).) By varying the source material, we also accelerated light ion beams, such as He-like fluorine, to over 5 MeV/nucleon.(M. Hegelich et al., Phys. Rev. Lett. 89, 085002 (2002).) From PIC simulations we understand the highest-energy and lowest-divergence proton acceleration as a transient laser-driven virtual cathode effect occurring at the target rear-surface. We have also confirmed the acceleration of ions from the front surface (A. Maksimchuk et al., Phys. Rev. Lett. 84, 4108 (2000).), which we find exhibits an intense low-energy component, but only a tenuous high-energy component, in agreement with PIC simulations. This work was performed with corporate support of General Atomics.

  19. Design of a submillimeter laser Thomson scattering system for measurement of ion temperature in SUMMA

    NASA Technical Reports Server (NTRS)

    Praddaude, H. C.; Woskoboinikow, P.

    1978-01-01

    A thorough discussion of submillimeter laser Thomson scattering for the measurement of ion temperature in plasmas is presented. This technique is very promising and work is being actively pursued on the high power lasers and receivers necessary for its implementation. In this report we perform an overall system analysis of the Thomson scattering technique aimed to: (1) identify problem areas; (2) establish specifications for the main components of the apparatus; (3) study signal processing alternatives and identify the optimum signal handling procedure. Because of its importance for the successful implementation of this technique, we also review the work presently being carried out on the optically pumped submillimeter CH3F and D2O lasers.

  20. Optimizing Laser-accelerated Ion Beams for a Collimated Neutron Source

    SciTech Connect

    C.L. Ellison and J. Fuchs

    2010-09-23

    High-flux neutrons for imaging and materials analysis applications have typically been provided by accelerator- and reactor-based neutron sources. A novel approach is to use ultraintense (>1018W/cm2) lasers to generate picosecond, collimated neutrons from a dual target configuration. In this article, the production capabilities of present and upcoming laser facilities are estimated while independently maximizing neutron yields and minimizing beam divergence. A Monte-Carlo code calculates angular and energy distributions of neutrons generated by D-D fusion events occurring within a deuterated target for a given incident beam of D+ ions. Tailoring of the incident distribution via laser parameters and microlens focusing modifies the emerging neutrons. Projected neutron yields and distributions are compared to conventional sources, yielding comparable on-target fluxes per discharge, shorter time resolution, larger neutron energies and greater collimation.

  1. Fiber Optic Picosecond Laser Pulse Transmission Line for Hydrogen Ion Beam Profile Measurement

    SciTech Connect

    Liu, Yun; Huang, Chunning; Aleksandrov, Alexander V

    2013-01-01

    We present a fiber optic laser pulse transmission line for non-intrusive longitudinal profile measurement of the hydrogen ion (H-) beam at the front-end of the Spallation Neutron Source (SNS) accelerator. The 80.5 MHz, 2.5 ps, multi-killowatt optical pulses are delivered to the accelerator beam line through a large mode area polarization maintaining optical fiber to ensure a high measurement stability. The transmission efficiency, output laser beam quality, pulse jitter and pulse width broadening over a 100-ft fiber line are experimentally investigated. A successful measurement of the H- beam microbunch (~130 ps) profile is obtained. Our experiment is the first demonstration of particle beam profile diagnostics using fiber optic laser pulse transmission line.

  2. Excitation mechanism in a hollow cathode He-Kr ion laser

    SciTech Connect

    Hazama, J.; Arai, T.; Goto, M.; Iijima, T.

    1995-12-31

    Pulsed laser operation in the afterglow of a positive column He-Kr discharge on the 469.4 nm (6s{sup 4}P{sub 5/2} {yields} 5p{sup 4}P{sub 5/2}) transition of Kr(II) was observed for the first time by Dana and Laure`s. It appears that the upper level of Kr(II) laser line is populated by the second kind collisions between He 2{sup 3}S metastable atoms and ground state Kr ions. CW oscillations on Kr(II) transitions have been obtained in a hollow cathode discharge. In this work, we have estimated the excitation mechanism for the upper state of 469.4 nm laser line from the measurements of the decay of endlight intensity in the hollow cathode He-Kr discharge.

  3. Fiber optic picosecond laser pulse transmission line for hydrogen ion beam longitudinal profile measurement.

    PubMed

    Huang, Chunning; Liu, Yun; Aleksandrov, Alexander

    2013-07-01

    We present a fiber optic laser pulse transmission line for nonintrusive longitudinal profile measurement of the hydrogen ion (H(-)) beam at the front-end of the Spallation Neutron Source accelerator. The 80.5 MHz, 2.5 ps, multikilowatt optical pulses are delivered to the accelerator beam line through a large-mode-area polarization-maintaining optical fiber to ensure high measurement stability. The transmission efficiency, output laser beam quality, pulse jitter, and pulse width broadening over a 30 m long fiber line are experimentally investigated. A successful measurement of the H(-) beam microbunch (~130 ps) profile is obtained. The experiment is the first demonstration to our knowledge of particle beam profile diagnostics using a fiber optic laser pulse transmission line.

  4. Monochromatic short pulse laser produced ion beam using a compact passive magnetic device

    SciTech Connect

    Chen, S. N.; Gauthier, M.; Higginson, D. P.; Dorard, S.; Marquès, J.-R.; Fuchs, J.; Mangia, F.; Atzeni, S.; Riquier, R.

    2014-04-15

    High-intensity laser accelerated protons and ions are emerging sources with complementary characteristics to those of conventional sources, namely high charge, high current, and short bunch duration, and therefore can be useful for dedicated applications. However, these beams exhibit a broadband energy spectrum when, for some experiments, monoenergetic beams are required. We present here an adaptation of conventional chicane devices in a compact form (10 cm × 20 cm) which enables selection of a specific energy interval from the broadband spectrum. This is achieved by employing magnetic fields to bend the trajectory of the laser produced proton beam through two slits in order to select the minimum and maximum beam energy. The device enables a production of a high current, short duration source with a reproducible output spectrum from short pulse laser produced charged particle beams.

  5. Monochromatic short pulse laser produced ion beam using a compact passive magnetic device.

    PubMed

    Chen, S N; Gauthier, M; Higginson, D P; Dorard, S; Mangia, F; Riquier, R; Atzeni, S; Marquès, J-R; Fuchs, J

    2014-04-01

    High-intensity laser accelerated protons and ions are emerging sources with complementary characteristics to those of conventional sources, namely high charge, high current, and short bunch duration, and therefore can be useful for dedicated applications. However, these beams exhibit a broadband energy spectrum when, for some experiments, monoenergetic beams are required. We present here an adaptation of conventional chicane devices in a compact form (10 cm × 20 cm) which enables selection of a specific energy interval from the broadband spectrum. This is achieved by employing magnetic fields to bend the trajectory of the laser produced proton beam through two slits in order to select the minimum and maximum beam energy. The device enables a production of a high current, short duration source with a reproducible output spectrum from short pulse laser produced charged particle beams. PMID:24784604

  6. Monochromatic short pulse laser produced ion beam using a compact passive magnetic device

    NASA Astrophysics Data System (ADS)

    Chen, S. N.; Gauthier, M.; Higginson, D. P.; Dorard, S.; Mangia, F.; Riquier, R.; Atzeni, S.; Marquès, J.-R.; Fuchs, J.

    2014-04-01

    High-intensity laser accelerated protons and ions are emerging sources with complementary characteristics to those of conventional sources, namely high charge, high current, and short bunch duration, and therefore can be useful for dedicated applications. However, these beams exhibit a broadband energy spectrum when, for some experiments, monoenergetic beams are required. We present here an adaptation of conventional chicane devices in a compact form (10 cm × 20 cm) which enables selection of a specific energy interval from the broadband spectrum. This is achieved by employing magnetic fields to bend the trajectory of the laser produced proton beam through two slits in order to select the minimum and maximum beam energy. The device enables a production of a high current, short duration source with a reproducible output spectrum from short pulse laser produced charged particle beams.

  7. Extending the applicability of an open-ring trap to perform experiments with a single laser-cooled ion

    SciTech Connect

    Cornejo, J. M.; Colombano, M.; Doménech, J.; Rodríguez, D.; Block, M.; Delahaye, P.

    2015-10-15

    A special ion trap was initially built up to perform β-ν correlation experiments with radioactive ions. The trap geometry is also well suited to perform experiments with laser-cooled ions, serving for the development of a new type of Penning trap, in the framework of the project TRAPSENSOR at the University of Granada. The goal of this project is to use a single {sup 40}Ca{sup +} ion as detector for single-ion mass spectrometry. Within this project and without any modification to the initial electrode configuration, it was possible to perform Doppler cooling on {sup 40}Ca{sup +} ions, starting from large clouds and reaching single ion sensitivity. This new feature of the trap might be important also for other experiments with ions produced at radioactive ion beam facilities. In this publication, the trap and the laser system will be described, together with their performance with respect to laser cooling applied to large ion clouds down to a single ion.

  8. Application of Laser Induced Breakdown Spectroscopy to Monitor Rare Earth Ions in Glass Matrix

    NASA Astrophysics Data System (ADS)

    Sharma, Prakash; Carter, Michael; Kumar, Akshaya

    2013-05-01

    The Laser Induced breakdown spectroscopy (LIBS) is a real time online technique that can be used to monitor the concentration of rare earth ions in amorphous glass matrix. This study has significant application in the glass industry where the composition of the glass can be monitored in real time using LIBS technology for quality control. The Eu3 + ions doped silicate glasses were developed via sol gel method. The glasses of varying molar percentages of Eu3 + (0.02, 0.05 and 0.08 mole percent), were prepared to study the effect of variation in concentration of Eu3 + ions on the LIBS signal and to calculate its limit of detection (LOD). The spectral assignment of the observed LIBS spectrum has been made. In order to find the maximum signal to noise ratio, we also recorded the intensity of LIBS signal for various integration start delay (ISD) time at a constant power of (pulsed Nd: YAG) laser. The ocean optics LIBS 2500plus spectrometer along with a Q switched Nd:YAG laser (Quantel, Big Sky) were used to record the LIBS spectrum.

  9. Controlling plasma distributions as driving forces for ion migration during fs laser writing

    NASA Astrophysics Data System (ADS)

    Teddy Fernandez, Toney; Siegel, Jan; Hoyo, Jesus; Sotillo, Belen; Fernandez, Paloma; Solis, Javier

    2015-04-01

    The properties of structures written inside dielectrics with high repetition rate femtosecond lasers are known to depend strongly on the complex interplay of a large number of writing parameters. Recently, ion migration within the laser-excited volume has been identified as a powerful mechanism for changing the local element distribution and producing efficient optical waveguides. In this work it is shown that the transient plasma distribution induced during laser irradiation is a reliable monitor for predicting the final refractive index distribution of the waveguide caused by ion migration. By performing in situ plasma emission microscopy during the writing process inside a La-phosphate glass it is found that the long axis of the plasma distribution determines the axis of ion migration, being responsible for the local refractive index increase. This observation is also valid when strong positive or negative spherical aberration is induced, greatly deforming the focal volume and inverting the index profile. Even subtle changes in the writing conditions, such as an inversion of the writing direction (quill writing effect), show up in the form of a modified plasma distribution, which manifests as a modified index distribution. Finally, it is shown that the superior control over the waveguide properties employing the slit shaping technique is caused by the more confined plasma distribution produced. The underlying reasons for this unexpected result are discussed in terms of non-linear propagation and heat accumulation.

  10. Ion and laser microprobes applied to the measurement of corrosion produced hydrogen on a microscopic scale.

    NASA Technical Reports Server (NTRS)

    Gray, H. R.

    1972-01-01

    Use of an ion microprobe and a laser microprobe to measure concentrations of corrosion-produced hydrogen on a microscopic scale. Hydrogen concentrations of several thousand ppm were measured by both analytical techniques below corroded and fracture surfaces of hot salt stress corroded titanium alloy specimens. This extremely high concentration compares with only about 100 ppm hydrogen determined by standard vacuum fusion chemical analyses of bulk samples. Both the ion and laser microprobes were used to measure hydrogen concentration profiles in stepped intervals to substantial depths below the original corroded and fracture surfaces. For the ion microprobe, the area of local analysis was 22 microns in diameter and for the laser microprobe, the area of local analysis was about 300 microns in diameter. The segregation of hydrogen below fracture surfaces supports a previously proposed theory that corrosion-produced hydrogen is responsible for hot salt stress corrosion embrittlement and cracking of titanium alloys. These advanced analytical techniques suggest great potential for many areas of stress corrosion and hydrogen embrittlement research, quality control, and field inspection of corrosion problems. For example, it appears possible that a contour map of hydrogen distribution at notch roots and crack tips could be quantitatively determined. Such information would be useful in substantiating current theories of stress corrosion and hydrogen embrittlement.

  11. Electron and Ion Emission from Clusters exposed to Strong Laser Fields

    NASA Astrophysics Data System (ADS)

    Tiggesbämker, Josef

    2006-03-01

    When clusters interact with intense optical laser pulses energetic and highly charged atomic fragment ions e.g. are generated^1. In contrast to atoms the efficiency of the process could be enhanced by choosing a pair of optical delayed pulses instead of a single but more intense femtosecond pulse^2. In metals the stronger charging of the clusters can qualitatively be explained by a plasmon enhanced ionization process. We extended our studies and have made a compared analysis of the emission of highly charged ions and energetic electrons the interaction dynamics of intense femtosecond laser fields with nanometer-sized silver clusters. Using a pair of laser pulses with variable optical delay the time-dependent cluster response is resolved. A dramatic increase both in the atomic charge state of the ions and the maximum electron kinetic energy is observed for a certain delay of the pulses. Corresponding Vlasov calculations on a metal cluster model system indicate that enhanced cluster ionization as well as the generation of fast electrons coincide with resonant plasmon excitation.^3 *L. Köller, M. Schumacher, J. Köhn, S. Teuber, J. Tiggesbäumker, and K.-H. Meiwes-Broer, Phys. Rev. Lett. 82, 3783 (1999). *T. Döppner, Th. Fennel, Th. Diederich, J. Tiggesb äumker, and K.-H. Meiwes-Broer, Phys. Rev. Lett. 94, 013401 (2005). *Th. Fennel, G.F. Bertsch, and K.-H. Meiwes-Broer, Eur. Phys. J. D 29, 367 (2004).

  12. Nonequilibrium properties of trapped ions under sudden application of a laser

    NASA Astrophysics Data System (ADS)

    Cifuentes, A. A.; Nicacio, F.; Paternostro, M.; Semião, F. L.

    2016-07-01

    Coherent quantum-state manipulation of trapped ions using classical laser fields is a trademark of modern quantum technologies. In this work, we study aspects of work statistics and irreversibility in a single trapped ion due to sudden interaction with the impinging laser. This is clearly an out-of-equilibrium process where work is performed through illumination of an ion by the laser. Starting with the explicit evaluation of the first moments of the work distribution, we proceed to a careful analysis of irreversibility as quantified by the nonequilibrium lag. The treatment employed here is not restricted to the Lamb-Dicke limit, which allows us to investigate the interplay between nonlinearities and irreversibility. We show that in these multiquantum or sideband regimes, variation of the Lamb-Dicke parameter causes a nonmonotonic behavior of the irreversibility indicator. Counterintuitively, we find a working point where nonlinearity helps reversibility, making the sudden quench of the Hamiltonian closer to what would have been obtained quasistatically and isothermally.

  13. Tetravalent Chromium (Cr(4+)) as Laser-Active Ion for Tunable Solid-State Lasers

    NASA Technical Reports Server (NTRS)

    Seas, A.; Petricevic, V.; Alfano, Robert R.

    1992-01-01

    During 10/31/91 - 3/31/92, the following summarizes are major accomplishments: (1) numerical modeling of the four mirror astigmatically compensated, Z-fold cavity was performed; and (2) the simulation revealed several design parameters to be used for the construction of a femtosecond forsterite laser.

  14. Resonant absorption effects induced by polarized laser light irradiating thin foils in the TNSA regime of ion acceleration

    NASA Astrophysics Data System (ADS)

    Torrisi, L.; Badziak, J.; Rosinski, M.; Zaras-Szydlowska, A.; Pfeifer, M.; Torrisi, A.

    2016-04-01

    Thin foils were irradiated by short pulsed lasers at intensities of 1016-19W/cm2 in order to produce non-equilibrium plasmas and ion acceleration from the target-normal-sheath-acceleration (TNSA) regime. Ion acceleration in forward direction was measured by SiC detectors and ion collectors used in the time-of-flight configuration. Laser irradiations were employed using p-polarized light at different incidence angles with respect to the target surface and at different focal distances from the target surface. Measurements demonstrate that resonant absorption effects, due to the plasma wave excitations, enhance the plasma temperature and the ion acceleration with respect to those performed without to use of p-polarized light. Dependences of the ion flux characteristics on the laser energy, wavelength, focal distance and incidence angle will be reported and discussed.

  15. Investigation of surface characteristics evolution and laser damage performance of fused silica during ion-beam sputtering

    NASA Astrophysics Data System (ADS)

    Xu, Mingjin; Dai, Yifan; Zhou, Lin; Shi, Feng; Wan, Wen; Xie, Xuhui; Sui, Tingting

    2016-08-01

    Surface characteristics have great influence on the optical properties especially the laser radiation resistivity of optics. In this paper, the surface characteristics evolutions of fused silica during ion-beam sputtering and their effects on the laser damage performance were investigated. The results show that roughness change is strongly removal depth dependent and a super-smooth surface (0.25 nm RMS) can be obtained by the ion-induced smoothing effect. The concentration of metal impurities (especially Ce element) in subsurface can be effectively decreased after the removal of polishing re-deposition layer. During ion-beam sputtering process, the plastic scratches can be removed while the brittle cracks can be broadened and passivated without increase in the depth direction. Laser damage threshold of fused silica improved by 36% after ion-beam sputtering treatment. Research results have a guiding significance for ion-beam sputtering process technology of fused silica optics.

  16. Reduction of angular divergence of laser-driven ion beams during their acceleration and transport

    NASA Astrophysics Data System (ADS)

    Zakova, M.; Pšikal, Jan; Margarone, Daniele; Maggiore, Mario; Korn, G.

    2015-05-01

    Laser plasma physics is a field of big interest because of its implications in basic science, fast ignition, medicine (i.e. hadrontherapy), astrophysics, material science, particle acceleration etc. 100-MeV class protons accelerated from the interaction of a short laser pulse with a thin target have been demonstrated. With continuing development of laser technology, greater and greater energies are expected, therefore projects focusing on various applications are being formed, e.g. ELIMAIA (ELI Multidisciplinary Applications of laser-Ion Acceleration). One of the main characteristic and crucial disadvantage of ion beams accelerated by ultra-short intense laser pulses is their large divergence, not suitable for the most of applications. In this paper two ways how to decrease beam divergence are proposed. Firstly, impact of different design of targets on beam divergence is studied by using 2D Particlein-cell simulations (PIC). Namely, various types of targets include at foils, curved foil and foils with diverse microstructures. Obtained results show that well-designed microstructures, i.e. a hole in the center of the target, can produce proton beam with the lowest divergence. Moreover, the particle beam accelerated from a curved foil has lower divergence compared to the beam from a flat foil. Secondly, another proposed method for the divergence reduction is using of a magnetic solenoid. The trajectories of the laser accelerated particles passing through the solenoid are modeled in a simple Matlab program. Results from PIC simulations are used as input in the program. The divergence is controlled by optimizing the magnetic field inside the solenoid and installing an aperture in front of the device.

  17. Generation of high currents of carbon ions with the use of subnanosecond near-infrared laser pulses

    SciTech Connect

    Krasa, J.; Velyhan, A.; Margarone, D.; Krousky, E.; Skala, J.; Laska, L.; Jungwirth, K.; Rohlena, K.; Ullschmied, J.

    2010-02-15

    Emission of carbon currents reaching values up to 2 A/cm{sup 2} at a distance of 1 m from the laser ion source driven by the subnanosecond Prague Asterix Laser System operated at a fundamental wavelength of 1315 nm is reported. Graphite targets were exposed to intensities up to 5x10{sup 16} W/cm{sup 2} varying both the laser energy and the position of the laser beam focus with respect to the target surface. The maximum energy gain of carbon ions was {approx_equal}1 MeV/u. At high laser intensities the shape of time-of-flight spectra is also formed by plasma outbursts, whose growth correlates with the oscillatory self-focusing of the laser beam.

  18. Internal Energy Deposition for Low Energy, Femtosecond Laser Vaporization and Nanospray Post-ionization Mass Spectrometry using Thermometer Ions

    NASA Astrophysics Data System (ADS)

    Flanigan, Paul M.; Shi, Fengjian; Archer, Jieutonne J.; Levis, Robert J.

    2015-05-01

    The internal energy of p-substituted benzylpyridinium ions after laser vaporization using low energy, femtosecond duration laser pulses of wavelengths 800 and 1042 nm was determined using the survival yield method. Laser vaporization of dried benzylpyridinium ions from metal slides into a buffered nanospray with 75 μJ, 800 nm laser pulses resulted in a higher extent of fragmentation than conventional nanospray due to the presence of a two-photon resonance fragmentation pathway. Using higher energy 800 nm laser pulses (280 and 505 μJ) led to decreased survival yields for the four different dried benzylpyridinium ions. Analyzing dried thermometer ions with 46.5 μJ, 1042 nm pulse-bursts resulted in little fragmentation and mean internal energy distributions equivalent to nanospray, which is attributable to the absence of a two-photon resonance that occurs with higher energy, 800 nm laser pulses. Vaporization of thermometer ions from solution with either 800 nm or 1042 nm laser pulses resulted in comparable internal energy distributions to nanospray ionization.

  19. Favorable target positions for intense laser acceleration of electrons in hydrogen-like, highly-charged ions

    SciTech Connect

    Pi, Liang-Wen; Starace, Anthony F.; Hu, S. X.

    2015-09-15

    Classical relativistic Monte Carlo simulations of petawatt laser acceleration of electrons bound initially in hydrogen-like, highly-charged ions show that both the angles and energies of the laser-accelerated electrons depend on the initial ion positions with respect to the laser focus. Electrons bound in ions located after the laser focus generally acquire higher (≈GeV) energies and are ejected at smaller angles with respect to the laser beam. Our simulations assume a tightly-focused linearly-polarized laser pulse with intensity approaching 10{sup 22 }W/cm{sup 2}. Up to fifth order corrections to the paraxial approximation of the laser field in the focal region are taken into account. In addition to the laser intensity, the Rayleigh length in the focal region is shown to play a significant role in maximizing the final energy of the accelerated electrons. Results are presented for both Ne{sup 9+} and Ar{sup 17+} target ions.

  20. Understanding plume splitting of laser ablated plasma: A view from ion distribution dynamics

    SciTech Connect

    Wu, Jian; Li, Xingwen; Wei, Wenfu; Jia, Shenli; Qiu, Aici

    2013-11-15

    Plume splitting in low-pressure ambient air was understood in view of ion distribution dynamics from the laser ablated Al plasma (1064 nm 0.57 J/mm{sup 2}) by combining fast photography and spatially resolved spectroscopy. In the beginning, the spectral lines were mainly from the Al III ion. Then, the Bragg peak in stopping power of the ambient gas to Al III could be the dominant reason for the enhanced emission from the fast moving part, and the recombination of Al III to Al I-II ions near the target surface was response to the radiations from the slow moving/stationary part. As the ambient gas pressure increased, stopping distances of the Al III decreased, and radiation from the air ions became pronounced. The laser shadowgraph image at 1100 Pa indicated that the shock wave front located between the fast moving and slow moving parts. Electron densities of the fast moving plasma, which peaked at the plasma front, were on the order of 10{sup 16} cm{sup −3}, and the electron temperatures were 2–3 eV.

  1. Synthesis of graphene and graphene nanostructures by ion implantation and pulsed laser annealing

    NASA Astrophysics Data System (ADS)

    Wang, Xiaotie; Berke, Kara; Rudawski, Nicholas G.; Venkatachalam, Dinesh K.; Elliman, Robert G.; Fridmann, Joel; Hebard, Arthur F.; Ren, Fan; Gila, Brent P.; Appleton, Bill R.

    2016-07-01

    In this paper, we report a systematic study that shows how the numerous processing parameters associated with ion implantation (II) and pulsed laser annealing (PLA) can be manipulated to control the quantity and quality of graphene (G), few-layer graphene (FLG), and other carbon nanostructures selectively synthesized in crystalline SiC (c-SiC). Controlled implantations of Si- plus C- and Au+ ions in c-SiC showed that both the thickness of the amorphous layer formed by ion damage and the doping effect of the implanted Au enhance the formation of G and FLG during PLA. The relative contributions of the amorphous and doping effects were studied separately, and thermal simulation calculations were used to estimate surface temperatures and to help understand the phase changes occurring during PLA. In addition to the amorphous layer thickness and catalytic doping effects, other enhancement effects were found to depend on other ion species, the annealing environment, PLA fluence and number of pulses, and even laser frequency. Optimum II and PLA conditions are identified and possible mechanisms for selective synthesis of G, FLG, and carbon nanostructures are discussed.

  2. Beam extraction from a laser-driven multicharged ion source (abstract)

    NASA Astrophysics Data System (ADS)

    Anderson, O. A.; Logan, B. Grant

    1998-02-01

    A newly proposed type of multicharged ion source has several potential advantages over existing types and a number of useful applications. The basic principle is that multiphoton absorption in an intense uniform laser focus can give multiple charge states of high purity (Ref. Reference 1). Thus, charge state separation downstream is simplified or made unnecessary. Another advantage is that large currents (hundreds of amperes) can be extracted. This type of source could be used for heavy-ion fusion drivers (see Ref. Reference 1) or storage rings. There are also industrial application such as materials processing. We describe conceptual design studies for several specific cases. For example, we discuss extraction and focusing of a 4.1 MV, 144 A beam of Xe16+ ions from an expanding plasma created by an intense laser. The maximum duration of the beam pulse is determined by the total charge in the plasma, while the practical pulse length is determined by the range of plasma radii over which good beam optics can be achieved. The initially diverging beam can be refocused to a small radius or made parallel by a combination of electrostatic and solenoid focusing. Our design studies are carried out first with an envelope code to determine the proper focusing parameters and then with a self-consistent particle code to optimize the beam quality. We present results from both codes and discuss several applications of this type of ion source.

  3. Brominated Tyrosine and Polyelectrolyte Multilayer Analysis by Laser Desorption VUV Postionization and Secondary Ion Mass Spectrometry

    SciTech Connect

    University of Illinois at Chicago; Blaze, Melvin M. T.; Takahashi, Lynelle; Zhou, Jia; Ahmed, Musahid; Gasper, Gerald; Pleticha, F. Douglas; Hanley, Luke

    2011-03-14

    The small molecular analyte 3,5-dibromotyrosine (Br2Y) and chitosan-alginate polyelectrolyte multilayers (PEM) with and without adsorbed Br2Y were analyzed by laser desorption postionization mass spectrometry (LDPI-MS). LDPI-MS using 7.87 eV laser and tunable 8 ? 12.5 eV synchrotron vacuum ultraviolet (VUV) radiation found that desorption of clusters from Br2Y films allowed detection by≤8 eV single photon ionization. Thermal desorption and electronic structure calculations determined the ionization energy of Br2Y to be ~;;8.3?0.1 eV and further indicated that the lower ionization energies of clusters permitted their detection at≤8 eV photon energies. However, single photon ionization could only detect Br2Y adsorbed within PEMs when using either higher photon energies or matrix addition to the sample. All samples were also analyzed by 25 keV Bi3 + secondary ion mass spectrometry (SIMS), with the negative ion spectra showing strong parent ion signal which complemented that observed by LDPI-MS. The negative ion SIMS depended strongly on the high electron affinity of this specific analyte and the analyte?s condensed phase environment.

  4. Behavior of moving plasma in solenoidal magnetic field in a laser ion source.

    PubMed

    Ikeda, S; Takahashi, K; Okamura, M; Horioka, K

    2016-02-01

    In a laser ion source, a solenoidal magnetic field is useful to guide the plasma and to control the extracted beam current. However, the behavior of the plasma drifting in the magnetic field has not been well understood. Therefore, to investigate the behavior, we measured the plasma ion current and the total charge within a single pulse in the solenoid by changing the distance from the entrance of the solenoid to a detector. We observed that the decrease of the total charge along the distance became smaller as the magnetic field became larger and then the charge became almost constant with a certain magnetic flux density. The results indicate that the transverse spreading speed of the plasma decreased with increasing the field and the plasma was confined transversely with the magnetic flux density. We found that the reason of the confinement was not magnetization of ions but an influence induced by electrons. PMID:26931973

  5. Behavior of moving plasma in solenoidal magnetic field in a laser ion source.

    PubMed

    Ikeda, S; Takahashi, K; Okamura, M; Horioka, K

    2016-02-01

    In a laser ion source, a solenoidal magnetic field is useful to guide the plasma and to control the extracted beam current. However, the behavior of the plasma drifting in the magnetic field has not been well understood. Therefore, to investigate the behavior, we measured the plasma ion current and the total charge within a single pulse in the solenoid by changing the distance from the entrance of the solenoid to a detector. We observed that the decrease of the total charge along the distance became smaller as the magnetic field became larger and then the charge became almost constant with a certain magnetic flux density. The results indicate that the transverse spreading speed of the plasma decreased with increasing the field and the plasma was confined transversely with the magnetic flux density. We found that the reason of the confinement was not magnetization of ions but an influence induced by electrons.

  6. Electron energy transport in ion waves and its relevance to laser-produced plasmas

    SciTech Connect

    Bell, A.R.

    1983-01-01

    Electron energy transport in plasmas is examined in the context of ion waves which are intermediate between collisionless isothermal ion acoustic waves and collisional adiabatic sound waves. The conductivity is found to be much less than the Spitzer-Haerm result for wavelengths less than 1000 electron mean free paths. This is expected to be relevant to laser-produced ablating plasmas in which the temperature can vary considerably over a distance of 10 to 100 mean free paths. The reduction in conductivity is independent of the wave amplitude thus differing from the reduction due to saturation found recently by numerical solution of the Fokker--Planck equation. At short wavelengths the heat flow approaches an upper limit which depends on the phase velocity of the wave. Diffusive ion wave damping is strong over a large range of wavelengths.

  7. Relativistically Induced Transparency Acceleration (RITA) - laser-plasma accelerated quasi-monoenergetic GeV ion-beams with existing lasers?

    NASA Astrophysics Data System (ADS)

    Sahai, Aakash A.

    2013-10-01

    Laser-plasma ion accelerators have the potential to produce beams with unprecedented characteristics of ultra-short bunch lengths (100s of fs) and high bunch-charge (1010 particles) over acceleration length of about 100 microns. However, creating and controlling mono-energetic bunches while accelerating to high-energies has been a challenge. If high-energy mono-energetic beams can be demonstrated with minimal post-processing, laser (ω0)-plasma (ωpe) ion accelerators may be used in a wide-range of applications such as cancer hadron-therapy, medical isotope production, neutron generation, radiography and high-energy density science. Here we demonstrate using analysis and simulations that using relativistic intensity laser-pulses and heavy-ion (Mi ×me) targets doped with a proton (or light-ion) species (mp ×me) of trace density (at least an order of magnitude below the cold critical density) we can scale up the energy of quasi-mono-energetically accelerated proton (or light-ion) beams while controlling their energy, charge and energy spectrum. This is achieved by controlling the laser propagation into an overdense (ω0 <ωpeγ = 1) increasing plasma density gradient by incrementally inducing relativistic electron quiver and thereby rendering them transparent to the laser while the heavy-ions are immobile. Ions do not directly interact with ultra-short laser that is much shorter in duration than their characteristic time-scale (τp <<√{mp} /ω0 <<√{Mi} /ω0). For a rising laser intensity envelope, increasing relativistic quiver controls laser propagation beyond the cold critical density. For increasing plasma density (ωpe2 (x)), laser penetrates into higher density and is shielded, stopped and reflected where ωpe2 (x) / γ (x , t) =ω02 . In addition to the laser quivering the electrons, it also ponderomotively drives (Fp 1/γ∇za2) them forward longitudinally, creating a constriction of snowplowed e-s. The resulting longitudinal e--displacement from

  8. Reaction ion etching process for improving laser damage resistance of fused silica optical surface.

    PubMed

    Sun, Laixi; Liu, Hongjie; Huang, Jin; Ye, Xin; Xia, Handing; Li, Qingzhi; Jiang, Xiaodong; Wu, Weidong; Yang, Liming; Zheng, Wanguo

    2016-01-11

    Laser induced damage of fused silica optics occurs primarily on optical surface or subsurface resulting from various defects produced during polishing/grinding process. Many new kinds of surface treatment processes are explored to remove or control the defects on fused silica surface. In this study, we report a new application of reaction ion etching (RIE)-based surface treatment process for manufacture of high quality fused silica optics. The influence of RIE processes on laser damage resistance as a function of etching depth and the evolution of typical defects which are associated with laser damage performance were investigated. The results show that the impurity element defects and subsurface damage on the samples surface were efficiently removed and prevented. Pure silica surface with relatively single-stable stoichiometry and low carbon atomic concentration was created during the etching. The laser damage resistance of the etched samples increased dramatically. The increase of roughness and ODC point defect with deeper etching are believed to be the main factors to limit further increase of the damage resistance of fused silica. The study is expected to contribute to the development of fused silica optics with high resistance to laser induced degradation in the future. PMID:26832251

  9. Laser acceleration of protons using multi-ion plasma gaseous targets

    SciTech Connect

    Liu, Tung -Chang; Shao, Xi; Liu, Chuan -Sheng; Eliasson, Bengt; W. T. Hill, III; Wang, Jyhpyng; Chen, Shih -Hung

    2015-02-01

    We present a theoretical and numerical study of a novel acceleration scheme by applying a combination of laser radiation pressure and shielded Coulomb repulsion in laser acceleration of protons in multi-species gaseous targets. By using a circularly polarized CO₂ laser pulse with a wavelength of 10 μm—much greater than that of a Ti: Sapphire laser—the critical density is significantly reduced, and a high-pressure gaseous target can be used to achieve an overdense plasma. This gives us a larger degree of freedom in selecting the target compounds or mixtures, as well as their density and thickness profiles. By impinging such a laser beam on a carbon–hydrogen target, the gaseous target is first compressed and accelerated by radiation pressure until the electron layer disrupts, after which the protons are further accelerated by the electron-shielded carbon ion layer. An 80 MeV quasi-monoenergetic proton beam can be generated using a half-sine shaped laser beam with a peak power of 70 TW and a pulse duration of 150 wave periods.

  10. Laser acceleration of protons using multi-ion plasma gaseous targets

    DOE PAGES

    Liu, Tung -Chang; Shao, Xi; Liu, Chuan -Sheng; Eliasson, Bengt; W. T. Hill, III; Wang, Jyhpyng; Chen, Shih -Hung

    2015-02-01

    We present a theoretical and numerical study of a novel acceleration scheme by applying a combination of laser radiation pressure and shielded Coulomb repulsion in laser acceleration of protons in multi-species gaseous targets. By using a circularly polarized CO₂ laser pulse with a wavelength of 10 μm—much greater than that of a Ti: Sapphire laser—the critical density is significantly reduced, and a high-pressure gaseous target can be used to achieve an overdense plasma. This gives us a larger degree of freedom in selecting the target compounds or mixtures, as well as their density and thickness profiles. By impinging such amore » laser beam on a carbon–hydrogen target, the gaseous target is first compressed and accelerated by radiation pressure until the electron layer disrupts, after which the protons are further accelerated by the electron-shielded carbon ion layer. An 80 MeV quasi-monoenergetic proton beam can be generated using a half-sine shaped laser beam with a peak power of 70 TW and a pulse duration of 150 wave periods.« less

  11. Universal Scalings for Direct Laser Acceleration of Relativistic Electrons in Ion Channels

    NASA Astrophysics Data System (ADS)

    Khudik, Vladimir; Arefiev, Alexey; Zhang, Xi; Shvets, Gennady

    2015-11-01

    Direct Laser Acceleration (DLA) of electrons in ion channels is investigated in the general case when the laser phase velocity is greater or equal to the speed of light, and the electrons execute a fully three-dimensional trajectory inside the focusing channel. In the paraxial limit of electron motion (mostly forward), we develop an analytic theory that provides an accurate estimate of the maximum possible energy gain of the electrons as a function of their initial conditions and laser parameters. Some of the counter-intuitive predictions validated via particle simulations include the emergence of the phase space barriers that prevent electrons from getting accelerated, and the threshold-like dependence of the energy on the initial conditions. The predictive power of the theory is demonstrated by identifying the laser-plasma parameters for the electron acceleration through the resonant interaction between the third harmonic of betatron oscillations and the laser wave. Possible experimental signatures of the high-order resonances will be discussed. This work was supported by DOE grants DESC0007889 and DE-SC0010622, and by an AFOSR grant FA9550-14-1-0045.

  12. Simulations of radiation pressure ion acceleration with the VEGA Petawatt laser

    NASA Astrophysics Data System (ADS)

    Stockhausen, Luca C.; Torres, Ricardo; Conejero Jarque, Enrique

    2016-09-01

    The Spanish Pulsed Laser Centre (CLPU) is a new high-power laser facility for users. Its main system, VEGA, is a CPA Ti:Sapphire laser which, in its final phase, will be able to reach Petawatt peak powers in pulses of 30 fs with a pulse contrast of 1 :1010 at 1 ps. The extremely low level of pre-pulse intensity makes this system ideally suited for studying the laser interaction with ultrathin targets. We have used the particle-in-cell (PIC) code OSIRIS to carry out 2D simulations of the acceleration of ions from ultrathin solid targets under the unique conditions provided by VEGA, with laser intensities up to 1022 W cm-2 impinging normally on 20 - 60 nm thick overdense plasmas, with different polarizations and pre-plasma scale lengths. We show how signatures of the radiation pressure-dominated regime, such as layer compression and bunch formation, are only present with circular polarization. By passively shaping the density gradient of the plasma, we demonstrate an enhancement in peak energy up to tens of MeV and monoenergetic features. On the contrary linear polarization at the same intensity level causes the target to blow up, resulting in much lower energies and broader spectra. One limiting factor of Radiation Pressure Acceleration is the development of Rayleigh-Taylor like instabilities at the interface of the plasma and photon fluid. This results in the formation of bubbles in the spatial profile of laser-accelerated proton beams. These structures were previously evidenced both experimentally and theoretically. We have performed 2D simulations to characterize this bubble-like structure and report on the dependency on laser and target parameters.

  13. Simulations of ion acceleration from ultrathin targets with the VEGA petawatt laser

    NASA Astrophysics Data System (ADS)

    Stockhausen, Luca C.; Torres, Ricardo; Conejero Jarque, Enrique

    2015-05-01

    The Spanish Pulsed Laser Centre (CLPU) is a new high-power laser facility for users. Its main system, VEGA, is a CPA Ti:Sapphire laser which, in its final phase, will be able to reach petawatt peak powers in pulses of 30 fs with a pulse contrast of 1 : 1010 at 1 ps. The extremely low level of pre-pulse intensity makes this system ideally suited for studying the laser interaction with ultrathin targets. We have used the particle-in-cell (PIC) code OSIRIS to carry out 2D simulations of the acceleration of ions from ultrathin solid targets under the unique conditions provided by VEGA, with laser intensities up to 1022Wcm-2 impinging normally on 5 - 40 nm thick overdense plasmas, with different polarizations and pre-plasma scale lengths. We show how signatures of the radiation pressure dominated regime, such as layer compression and bunch formation, are only present with circular polarization. By passively shaping the density gradient of the plasma, we demonstrate an enhancement in peak energy up to tens of MeV and monoenergetic features. On the contrary linear polarization at the same intensity level causes the target to blow up, resulting in much lower energies and broader spectra. One limiting factor of Radiation Pressure Acceleration is the development of Rayleigh-Taylor like instabilities at the interface of the plasma and photon fluid. This results in the formation of bubbles in the spatial profile of laser-accelerated proton beams. These structures were previously evidenced both experimentally and theoretically. We have performed 2D simulations to characterize this bubble-like structure and report on the dependency on laser and target parameters.

  14. Ion-to-Neutral Ratios and Thermal Proton Transfer in Matrix-Assisted Laser Desorption/Ionization

    NASA Astrophysics Data System (ADS)

    Lu, I.-Chung; Chu, Kuan Yu; Lin, Chih-Yuan; Wu, Shang-Yun; Dyakov, Yuri A.; Chen, Jien-Lian; Gray-Weale, Angus; Lee, Yuan-Tseh; Ni, Chi-Kung

    2015-07-01

    The ion-to-neutral ratios of four commonly used solid matrices, α-cyano-4-hydroxycinnamic acid (CHCA), 2,5-dihydroxybenzoic acid (2,5-DHB), sinapinic acid (SA), and ferulic acid (FA) in matrix-assisted laser desorption/ionization (MALDI) at 355 nm are reported. Ions are measured using a time-of-flight mass spectrometer combined with a time-sliced ion imaging detector. Neutrals are measured using a rotatable quadrupole mass spectrometer. The ion-to-neutral ratios of CHCA are three orders of magnitude larger than those of the other matrices at the same laser fluence. The ion-to-neutral ratios predicted using the thermal proton transfer model are similar to the experimental measurements, indicating that thermal proton transfer reactions play a major role in generating ions in ultraviolet-MALDI.

  15. Ion-to-Neutral Ratios and Thermal Proton Transfer in Matrix-Assisted Laser Desorption/Ionization.

    PubMed

    Lu, I-Chung; Chu, Kuan Yu; Lin, Chih-Yuan; Wu, Shang-Yun; Dyakov, Yuri A; Chen, Jien-Lian; Gray-Weale, Angus; Lee, Yuan-Tseh; Ni, Chi-Kung

    2015-07-01

    The ion-to-neutral ratios of four commonly used solid matrices, α-cyano-4-hydroxycinnamic acid (CHCA), 2,5-dihydroxybenzoic acid (2,5-DHB), sinapinic acid (SA), and ferulic acid (FA) in matrix-assisted laser desorption/ionization (MALDI) at 355 nm are reported. Ions are measured using a time-of-flight mass spectrometer combined with a time-sliced ion imaging detector. Neutrals are measured using a rotatable quadrupole mass spectrometer. The ion-to-neutral ratios of CHCA are three orders of magnitude larger than those of the other matrices at the same laser fluence. The ion-to-neutral ratios predicted using the thermal proton transfer model are similar to the experimental measurements, indicating that thermal proton transfer reactions play a major role in generating ions in ultraviolet-MALDI.

  16. High-precision hyperfine structure measurement in slow atomic ion beams by collinear laser-rf double resonance

    SciTech Connect

    Amarjit Sen, Childs, W.J.; Goodman, L.S.

    1987-01-01

    A new collinear laser-ion beam apparatus for slow ions (1 to 1.5 keV) has been built for measuring the hyperfine structure of metastable levels of ions with laser-rf double resonance technique. Narrow linewidths of approx.60 kHz (FWHM) have been observed for the first time in such systems. As a first application the hyperfine structure of the 4f/sup 7/(/sup 8/S/sup 0/)5d /sup 9/D/sub J//sup 0/ metastable levels of /sup 151,153/Eu/sup +/ has been measured with high precision. 10 refs., 8 figs.

  17. A universal gate set on a Trapped-Ion Optical Qubit using a narrow linewidth Diode laser

    NASA Astrophysics Data System (ADS)

    Glickman, Yinnon; Akerman, Nitzan; Kotler, Shlomi; Kesselman, Anna; Ozeri, Roee

    2011-05-01

    Optical qubit states are encoded in the 5S1/2 ground state and the meta-stable 4D5/2 level in a single trapped 88Sr+ ion, connected by a narrow optical quadruple transition. A 674nm diode laser is frequency stabilized and narrowed to a line-width below 80 Hz. Using this laser we demonstrate a universal quantum gate-set as well as other coherent operations on the ions' internal and external degrees of freedom. Rabi flopping, Ramsey spectroscopy and ground state cooling of the qubit are performed. Using a bi-chromatic beam, two ion-qubits are entangled with a Sorenson-Molmer entangling gate scheme. The advantages and disadvantages of using a diode laser to this end are discussed. In particular, the contribution of fast phase noise, typical to diode laser systems, to off-resonance qubit excitation and gate error is analyzed.

  18. High performance compact magnetic spectrometers for energetic ion and electron measurement in ultra intense short pulse laser solid interactions

    SciTech Connect

    Chen, H; Link, A; van Maren, R; Patel, P; Shepherd, R; Wilks, S C; Beiersdorfer, P

    2008-05-08

    Ultra intense short pulse lasers incident on solid targets can generate relativistic electrons that then accelerate energetic protons and ions. These fast electrons and ions can effectively heat the solid target, beyond the region of direct laser interaction, and are vital to realizing the fast ignition concept. To study these energetic ions and electrons produced from the laser-target interactions, we have developed a range of spectrometers that can cover a large energy range (from less than 0.1 MeV to above 100 MeV). They are physically compact and feature high performance and low cost. We will present the basic design of these spectrometers and their test results from recent laser experiments.

  19. Shock ion acceleration by an ultrashort circularly polarized laser pulse via relativistic transparency in an exploded target.

    PubMed

    Kim, Young-Kuk; Cho, Myung-Hoon; Song, Hyung Seon; Kang, Teyoun; Park, Hyung Ju; Jung, Moon Youn; Hur, Min Sup

    2015-10-01

    We investigated ion acceleration by an electrostatic shock in an exploded target irradiated by an ultrashort, circularly polarized laser pulse by means of one- and three-dimensional particle-in-cell simulations. We discovered that the laser field penetrating via relativistic transparency (RT) rapidly heated the upstream electron plasma to enable the formation of a high-speed electrostatic shock. Owing to the RT-based rapid heating and the fast compression of the initial density spike by a circularly polarized pulse, a new regime of the shock ion acceleration driven by an ultrashort (20-40 fs), moderately intense (1-1.4 PW) laser pulse is envisaged. This regime enables more efficient shock ion acceleration under a limited total pulse energy than a linearly polarized pulse with crystal laser systems of λ∼1μm.

  20. Generation of heavy ion beams using femtosecond laser pulses in the target normal sheath acceleration and radiation pressure acceleration regimes

    NASA Astrophysics Data System (ADS)

    Petrov, G. M.; McGuffey, C.; Thomas, A. G. R.; Krushelnick, K.; Beg, F. N.

    2016-06-01

    Theoretical study of heavy ion acceleration from sub-micron gold foils irradiated by a short pulse laser is presented. Using two dimensional particle-in-cell simulations, the time history of the laser pulse is examined in order to get insight into the laser energy deposition and ion acceleration process. For laser pulses with intensity 3 × 10 21 W / cm 2 , duration 32 fs, focal spot size 5 μm, and energy 27 J, the calculated reflection, transmission, and coupling coefficients from a 20 nm foil are 80%, 5%, and 15%, respectively. The conversion efficiency into gold ions is 8%. Two highly collimated counter-propagating ion beams have been identified. The forward accelerated gold ions have average and maximum charge-to-mass ratio of 0.25 and 0.3, respectively, maximum normalized energy 25 MeV/nucleon, and flux 2 × 10 11 ions / sr . An analytical model was used to determine a range of foil thicknesses suitable for acceleration of gold ions in the radiation pressure acceleration regime and the onset of the target normal sheath acceleration regime. The numerical simulations and analytical model point to at least four technical challenges hindering the heavy ion acceleration: low charge-to-mass ratio, limited number of ions amenable to acceleration, delayed acceleration, and high reflectivity of the plasma. Finally, a regime suitable for heavy ion acceleration has been identified in an alternative approach by analyzing the energy absorption and distribution among participating species and scaling of conversion efficiency, maximum energy, and flux with laser intensity.