Crossed-beam velocity map imaging of collisional autoionization processes
NASA Astrophysics Data System (ADS)
Delmdahl, Ralph F.; Bakker, Bernard L. G.; Parker, David H.
2000-11-01
Applying the velocity map imaging technique Penning ion formation as well as generation of associative ions is observed in autoionizing collisions of metastable neon atoms (Ne* 2p5 3s 3P2,0) with ground state argon targets in a crossed molecular beam experiment. Metastable neon reactants are obtained by nozzle expansion through a dc discharge ring. The quality of the obtained results clearly demonstrates the suitability of this new, particularly straightforward experimental approach with respect to angle and kinetic energy resolved investigations of Penning processes in crossed-beam studies which are known to provide the highest level of detail.
Birth of a resonant attosecond wavepacket
NASA Astrophysics Data System (ADS)
Argenti, L.; Gruson, V.; Barreau, L.; Jimenez-Galan, A.; Risoud, F.; Caillat, J.; Maquet, A.; Carre, B.; Lepetit, F.; Hergott, J.-F.; Ruchon, T.; Taieb, R.; Martin, F.; Salieres, P.
2016-05-01
Both amplitude and phase are needed to characterize the dynamics of a wavepacket. However, such characterization is difficult when both attosecond and femtosecond timescales are involved, as it is the case for broadband photoionization to a continuum encompassing autoionizing states. Here we demonstrate that Rainbow RABBIT, a new attosecond interferometry, allows the measurement of amplitude and phase of a photoelectron wavepacket created through a Fano resonance with unprecedented precision. In the experiment, a tunable attosecond pulse train is combined with the fundamental laser pulse to induce two-photon transitions in helium via an intermediate autoionizing state. From the energy and time-delay resolved signal, we fully reconstruct the resonant electron wavepacket as it builds up in the continuum. Measurements accurately match the predictions of a new time-resolved multi-photon resonant model, known to reproduce ab initio calculations. This agreement confirms the potential of Rainbow RABBIT to investigate photoemission delays in ultrafast processes governed by electron correlation, as well as to control structured electron wavepackets. now at Univ. Central Florida, Orlando, FL (USA).
Photoelectron angular distributions from rotationally resolved autoionizing states of N 2
Chartrand, A. M.; McCormack, E. F.; Jacovella, U.; ...
2017-12-08
The single-photon, photoelectron-photoion coincidence spectrum of N 2 has been recorded at high (~1.5 cm -1) resolution in the region between the N 2 + X 2Σ g +, v + = 0 and 1 ionization thresholds by using a double imaging spectrometer and intense vacuum-ultraviolet light from the Synchrotron SOLEIL. This approach provides the relative photoionization cross section, the photoelectron energy distribution, and the photoelectron angular distribution as a function of photon energy. The region of interest contains autoionizing valence states, vibrationally autoionizing Rydberg states converging to vibrationally excited levels of the N 2 + X 2Σ g +more » ground state, and electronically autoionizing states converging to the N 2 + A 2Π and B 2Σ u + states. The wavelength resolution is sufficient to resolve rotational structure in the autoionizing states, but the electron energy resolution is insufficient to resolve rotational structure in the photoion spectrum. Here, a simplified approach based on multichannel quantum defect theory is used to predict the photoelectron angular distribution parameters, β, and the results are in reasonably good agreement with experiment.« less
NASA Astrophysics Data System (ADS)
Holland, D. M. P.; Shaw, D. A.
2014-01-01
The effect of vibrational autoionization on the H2+ X 2Σg+ v+ = 3, N+ state rotationally resolved photoelectron angular distributions and branching ratios has been investigated with a velocity map imaging spectrometer and synchrotron radiation. In photon excitation regions free from the influence of autoionizing Rydberg states, where direct ionization dominates, the photoelectron anisotropy parameter associated with the X 1Σg+ v″ = 0, N″ = 1 → X 2Σg+ v+ = 3, N+ = 1 transition has a value close to the theoretical maximum. However, in the vicinity of a Rydberg state, vibrational autoionization leads to a substantial reduction in anisotropy. The value of the anisotropy parameter associated with the S-branch of the photoelectron spectrum is found to be considerably higher than that predicted under the assumption that the outgoing electron can be represented solely as a p-wave. This suggests that the f-wave contribution must be taken into account to obtain a proper description of the photoionization dynamics. The observed variations in the rotationally resolved branching ratios, in the vicinity of an autoionizing resonance, depend upon the rotational level of the Rydberg state. The rotationally averaged photoelectron anisotropy parameters have been compared with the corresponding, previously calculated, theoretical results and reasonable agreement has been found. The influence of vibrational autoionization on the H2+ X 2Σg+ v+ = 0, 1, 2, 3 vibrational branching ratios has also been investigated, and the experimental results show that, in energy regions encompassing Rydberg states, these ratios deviate strongly from the Franck-Condon factors for direct ionization.
Analytical model for atomic resonant attosecond transient absorption
NASA Astrophysics Data System (ADS)
Cariker, C.; Kjellson, T.; Lindroth, E.; Argenti, L.
2017-04-01
Recent advancements in ultrafast laser technology have made it possible to probe electron dynamics in highly excited atomic states that autoionize on a femtosecond timescale, thus giving insight into the dynamics of Auger decay and its interference with the continuum. These experiments provide a stringent test for time-resolved analytical models of autoionization. Here we present a finite-pulse, multi-photon perturbative model which is used in conjunction with ab-initio structure calculations to predict the attosecond transient absorption spectrum (ATAS) of an atom above the ionization threshold. We apply this model to compute the ATAS of argon in the vicinity of the 3s-1 4 p resonance as a function of the time delay between an extreme ultraviolet (XUV) and an infrared (IR) pulse, as well as of the angle between their polarization. We show that by modulating the parameters of the IR pulse it is possible to control the dipolar coupling between neighboring states and hence the lineshape of the 3s-1 4 p resonance. NSF Grant No. 1607588.
Klinker, Markus; Marante, Carlos; Argenti, Luca; González-Vázquez, Jesús; Martín, Fernando
2018-02-15
Direct measurement of autoionization lifetimes by using time-resolved experimental techniques is a promising approach when energy-resolved spectroscopic methods do not work. Attosecond time-resolved experiments have recently provided the first quantitative determination of autoionization lifetimes of the lowest members of the well-known Hopfield series of resonances in N 2 . In this work, we have used the recently developed XCHEM approach to study photoionization of the N 2 molecule in the vicinity of these resonances. The XCHEM approach allows us to describe electron correlation in the molecular electronic continuum at a level similar to that provided by multireference configuration interaction methods in bound state calculations, a necessary condition to accurately describe autoionization, shakeup, and interchannel couplings occurring in this range of photon energies. Our results show that electron correlation leading to interchannel mixing is the main factor that determines the magnitude and shape of the N 2 photoionization cross sections, as well as the lifetimes of the Hopfield resonances. At variance with recent speculations, nonadiabatic effects do not seem to play a significant role. These conclusions are supported by the very good agreement between the calculated cross sections and those determined in synchrotron radiation and attosecond experiments.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Chartrand, A. M.; McCormack, E. F.; Jacovella, U.
The single-photon, photoelectron-photoion coincidence spectrum of N 2 has been recorded at high (~1.5 cm -1) resolution in the region between the N 2 + X 2Σ g +, v + = 0 and 1 ionization thresholds by using a double imaging spectrometer and intense vacuum-ultraviolet light from the Synchrotron SOLEIL. This approach provides the relative photoionization cross section, the photoelectron energy distribution, and the photoelectron angular distribution as a function of photon energy. The region of interest contains autoionizing valence states, vibrationally autoionizing Rydberg states converging to vibrationally excited levels of the N 2 + X 2Σ g +more » ground state, and electronically autoionizing states converging to the N 2 + A 2Π and B 2Σ u + states. The wavelength resolution is sufficient to resolve rotational structure in the autoionizing states, but the electron energy resolution is insufficient to resolve rotational structure in the photoion spectrum. Here, a simplified approach based on multichannel quantum defect theory is used to predict the photoelectron angular distribution parameters, β, and the results are in reasonably good agreement with experiment.« less
Eckstein, Martin; Yang, Chung-Hsin; Frassetto, Fabio; Poletto, Luca; Sansone, Giuseppe; Vrakking, Marc J J; Kornilov, Oleg
2016-04-22
Autoionizing Rydberg states of molecular N_{2} are studied using time-, energy-, and angular-resolved photoelectron spectroscopy. A femtosecond extreme ultraviolet pulse with a photon energy of 17.5 eV excites the resonance and a subsequent IR pulse ionizes the molecule before the autoionization takes place. The angular-resolved photoelectron spectra depend on pump-probe time delay and allow for the distinguishing of two electronic states contributing to the resonance. The lifetime of one of the contributions is determined to be 14±1 fs, while the lifetime of the other appears to be significantly shorter than the time resolution of the experiment. These observations suggest that the Rydberg states in this energy region are influenced by the effect of interference stabilization and merge into a complex resonance.
Time-frequency representation of autoionization dynamics in helium
NASA Astrophysics Data System (ADS)
Busto, D.; Barreau, L.; Isinger, M.; Turconi, M.; Alexandridi, C.; Harth, A.; Zhong, S.; Squibb, R. J.; Kroon, D.; Plogmaker, S.; Miranda, M.; Jiménez-Galán, Á.; Argenti, L.; Arnold, C. L.; Feifel, R.; Martín, F.; Gisselbrecht, M.; L'Huillier, A.; Salières, P.
2018-02-01
Autoionization, which results from the interference between direct photoionization and photoexcitation to a discrete state decaying to the continuum by configuration interaction, is a well known example of the important role of electron correlation in light-matter interaction. Information on this process can be obtained by studying the spectral, or equivalently, temporal complex amplitude of the ionized electron wave packet. Using an energy-resolved interferometric technique, we measure the spectral amplitude and phase of autoionized wave packets emitted via the sp2+ and sp3+ resonances in helium. These measurements allow us to reconstruct the corresponding temporal profiles by Fourier transform. In addition, applying various time-frequency representations, we observe the build-up of the wave packets in the continuum, monitor the instantaneous frequencies emitted at any time and disentangle the dynamics of the direct and resonant ionization channels.
Sommavilla, M; Merkt, F; Mezei, J Zs; Jungen, Ch
2016-02-28
Absorption and photoionization spectra of H2 have been recorded at a resolution of 0.09 and 0.04 cm(-1), respectively, between 125,600 cm(-1) and 126,000 cm(-1). The observed Rydberg states belong to series (n = 10 - 14) converging on the first vibrationally excited level of the X (2)Σ(g)(+) state of H2(+), and of lower members of series converging on higher vibrational levels. The observed resonances are characterized by the competition between autoionization, predissociation, and fluorescence. The unprecedented resolution of the present experimental data leads to a full characterization of the predissociation/autoionization profiles of many resonances that had not been resolved previously. Multichannel quantum defect theory is used to predict the line positions, widths, shapes, and intensities of the observed spectra and is found to yield quantitative agreement using previously determined quantum defect functions as the unique set of input parameters.
NASA Astrophysics Data System (ADS)
Jacobs, Verne L.
2017-06-01
This investigation has been devoted to the theoretical description and computer modeling of atomic processes giving rise to radiative emission in energetic electron and ion beam interactions and in laboratory plasmas. We are also interested in the effects of directed electron and ion collisions and of anisotropic electric and magnetic fields. In the kinetic-theory description, we treat excitation, de-excitation, ionization, and recombination in electron and ion encounters with partially ionized atomic systems, including the indirect contributions from processes involving autoionizing resonances. These fundamental collisional and electromagnetic interactions also provide particle and photon transport mechanisms. From the spectral perspective, the analysis of atomic radiative emission can reveal detailed information on the physical properties in the plasma environment, such as non-equilibrium electron and charge-state distributions as well as electric and magnetic field distributions. In this investigation, a reduced-density-matrix formulation is developed for the microscopic description of atomic electromagnetic interactions in the presence of environmental (collisional and radiative) relaxation and decoherence processes. Our central objective is a fundamental microscopic description of atomic electromagnetic processes, in which both bound-state and autoionization-resonance phenomena can be treated in a unified and self-consistent manner. The time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations of the reduced-density-matrix approach are developed in a unified and self-consistent manner. This is necessary for our ultimate goal of a systematic and self-consistent treatment of non-equilibrium (possibly coherent) atomic-state kinetics and high-resolution (possibly overlapping) spectral-line shapes. We thereby propose the introduction of a generalized collisional-radiative atomic-state kinetics model based on a reduced-density-matrix formulation. It will become apparent that the full atomic data needs for the precise modeling of extreme non-equilibrium plasma environments extend beyond the conventional radiative-transition-probability and collisional-cross-section data sets.
Attosecond-resolved photoionization of chiral molecules.
Beaulieu, S; Comby, A; Clergerie, A; Caillat, J; Descamps, D; Dudovich, N; Fabre, B; Géneaux, R; Légaré, F; Petit, S; Pons, B; Porat, G; Ruchon, T; Taïeb, R; Blanchet, V; Mairesse, Y
2017-12-08
Chiral light-matter interactions have been investigated for two centuries, leading to the discovery of many chiroptical processes used for discrimination of enantiomers. Whereas most chiroptical effects result from a response of bound electrons, photoionization can produce much stronger chiral signals that manifest as asymmetries in the angular distribution of the photoelectrons along the light-propagation axis. We implemented self-referenced attosecond photoelectron interferometry to measure the temporal profile of the forward and backward electron wave packets emitted upon photoionization of camphor by circularly polarized laser pulses. We measured a delay between electrons ejected forward and backward, which depends on the ejection angle and reaches 24 attoseconds. The asymmetric temporal shape of electron wave packets emitted through an autoionizing state further reveals the chiral character of strongly correlated electronic dynamics. Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.
Angle-resolved photoelectron spectroscopy of cyclopropane
NASA Astrophysics Data System (ADS)
Keller, P. R.; Taylor, J. W.; Carlson, Thomas A.; Whitley, T. A.; Grimm, F. A.
1985-10-01
The angular distribution parameter, β, determined for the valence orbitals (IP < 18 eV) of cyclopropane in the 10-30 eV photon energy range using dispersed polarized synchrotron radiation. The energy dependence of β for photoelectron energies between, 2 and 10 eV above threshold was found to be similar to those found previously for other σ orbitals. The effects of Jahn-Teller splitting on β for the 3e' orbital were found to be small but definitely present. The overall shape and magnitude of the β( hv) curve are, however, sufficiently for the different Jahn-Teller components that, for purposes of orbital assignments using β( hv) curves the shape and magnitude of the curves can be considered associated only with the initial state. Resonance photoionization features at a photon ener of ≈ 18 eV were observed in the 3e' and 3a' 1 orbitals and tentatively assigned to autoionization.
NASA Astrophysics Data System (ADS)
Martin, N. L. S.; Weaver, C. M.; Kim, B. N.; deHarak, B. A.; Zatsarinny, O.; Bartschat, K.
2018-05-01
Out-of-scattering-plane (e ,2 e ) measurements and calculations are reported for the three singlet helium 2 ℓ 2 ℓ' autoionizing levels, with 80, 100, 120, 150, and 488 eV incident-electron energies, and scattering angles 60∘, 50 .8∘ , 45∘, 39 .2∘ , and 20 .5∘ , respectively. The kinematics are the same in all cases: the momentum transfer is K =2.1 a.u., and ejected electrons are detected in a plane that contains the momentum-transfer direction and is perpendicular to the scattering plane. The results are presented as (e ,2 e ) angular distributions energy integrated over each level. They are compared with fully nonperturbative B -spline R -matrix and hybrid second-order distorted-wave + R -matrix calculations.
NASA Astrophysics Data System (ADS)
Farhat, Ahmad H.
This dissertation, which is in the area of atomic physics, concentrates on the study of the interaction between VUV-soft X-ray radiation and atoms in the gas phase. The main area of interest is the study of Auger decay in atoms utilizing the process known as the resonance Auger effect, where an inner shell electron is excited to an unfilled orbital followed by the ejection of an Auger electron. The measurements in this thesis were performed by using the high resolution Atomic, Molecular and Optical Physics undulator beam line, which utilizes a spherical grating monochromator at the Advanced Light Source at Lawrence Berkeley National Laboratory. The research focused on three rare gases, argon, krypton and xenon. For argon, high resolution angular-resolved measurements of the 2p → 4s, 3d, 4d resonant Auger lines have been achieved. By measuring photoelectron spectra simultaneously at two different angles using efficient time of flight spectrometers, the angular distributions anisotropy parameters β have been measured, and relative intensities have been evaluated for each of the resolved final ionic states. For krypton, the resonant Auger decay of all the photoexcited Kr 3d3/2,5/2-1 nl (n = 5-9) states have been studied using an angle resolved two dimensional photoelectron spectroscopic technique, in which the electron yield was measured as a function of both photon energy and electron kinetic energy. Angular distributions, spectator and shake probabilities have been derived for the Kr 3d-1np/to4s- 14p-1mp + e/sp- (n = 5-9, m = 5-11) resonance Auger decay. The results show that the spectator-core coupling is strong at lower n (n = 5,6) but it lessens for higher n, with a shake up of m = n + 1 preferred. Finally for xenon, the autoionization resonances and angular distribution of the 4d → 6p decay spectrum were studied utilizing the Auger resonant Raman effect. Using this technique, β parameters of almost all 5p4/ (3P,/ 1D,/ 1S) 6p final ionic states were determined. These results contribute to our understanding of atomic structure and dynamics of inner shell processes and hopefully will stimulate further experimental and theoretical work.
NASA Technical Reports Server (NTRS)
Currie, J. R.; Kissel, R. R.
1986-01-01
A system for the measurement of shaft angles is disclosed wherein a synchro resolver is sequentially pulsed, and alternately, a sine and then a cosine representative voltage output of it are sampled. Two like type, sine or cosine, succeeding outputs (V sub S1, V sub S2) are averaged and algebraically related to the opposite type output pulse (V sub c) occurring between the averaged pulses to provide a precise indication of the angle of a shaft coupled to the resolver at the instant of the occurrence of the intermediately occurring pulse (V sub c).
Femtosecond Photoelectron Imaging of Dissociating and Autoionizing States in Oxygen
NASA Astrophysics Data System (ADS)
Plunkett, Alexander; Sandhu, Arvinder
2017-04-01
Time-resolved photoelectron spectra from molecular oxygen have been recorded with high energy and time resolution using a velocity map imaging (VMI) spectrometer. High harmonics were used to prepare neutral Rydberg states converging to the c4Σu- ionic state. These states display both autoionization and predissociation. A femtosecond laser pulse centered at 780 nm was used to probe the system, ionizing both the excited molecular states and the predissociated neutral atomic fragments. Electrons were collected in the 0-3 eV range using a VMI spectrometer and their spectra were reconstructed using a Fast Onion-peeling algorithm. By looking at IR modification to the electron spectrum, new features are observed which could originate from long-range columbic interactions or previously unobserved molecular decay channels. Ongoing studies extend this technique to other systems exhibiting non-adiabatic dynamics. This work was supported by the U. S. Army Research Laboratory and the U. S. Army Research Office under Grant No. W911NF-14-1-0383.
Partially autoionizing states of atomic oxygen
NASA Technical Reports Server (NTRS)
Samson, J. A. R.; Petrosky, V. E.
1974-01-01
Certain Rydberg states and an intershell transition of atomic oxygen were shown to partially autoionize, and to produce emission spectra competitive with autoionization. These states are forbidden to autoionize on the basis of LS coupling; but they were observed both in emission spectroscopy and in photoelectron spectroscopy. The results explain an unidentified structure in the 584 Angstrom He I atomic O spectrum observed by previous investigators.
Observation of autoionization in O 2 by an electron-electron coincidence method
NASA Astrophysics Data System (ADS)
Doering, J. P.; Yang, J.; Cooper, J. W.
1995-01-01
A strong transition to an autoionizing stata has been observed in O 2 at 16.83 ± 0.11 eV by means of a new electron-electron conincidence method. The method uses the fact that electrons arising from autoionizing states appear at a constant energy loss corresponding to the excitation energy of the autoionizing state rather than at a constant ionization potential as do electrons produced by direct ionization. Comparison of the present data with previous photoionization studies suggests that the autoionizing O 2 state is the same state deduced to be responsible for abnormal vibrational intensities in the O 2+X 2Πg ground state when 16.85 eV Ne(I) photons are used. These electron-electron coincidence experiments provide a direct new method for the study of autoionization produced by electron impact.
Control integration concept for hypersonic cruise-turn maneuvers
NASA Technical Reports Server (NTRS)
Raney, David L.; Lallman, Frederick J.
1992-01-01
Piloting difficulties associated with conducting aircraft maneuvers in hypersonic flight are caused in part by the nonintuitive nature of the aircraft response and the stringent constraints anticipated on allowable angle of attack and dynamic pressure variations. An approach is documented that provides precise, coordinated maneuver control during excursions from a hypersonic cruise flight path and the necessary flight condition constraints. The approach is to achieve specified guidance commands by resolving altitude and cross range errors into a load factor and bank angle command by using a coordinate transformation that acts as an interface between outer and inner loop flight controls. This interface, referred to as a 'resolver', applies constraints on angle of attack and dynamic pressure perturbations while prioritizing altitude regulation over cross range. An unpiloted test simulation, in which the resolver was used to drive inner loop flight controls, produced time histories of responses to guidance commands and atmospheric disturbances at Mach numbers of 6, 10, 15, and 20. Angle of attack and throttle perturbation constraints, combined with high speed flight effects and the desire to maintain constant dynamic pressure, significantly impact the maneuver envelope for a hypersonic vehicle.
A 72 × 60 Angle-Sensitive SPAD Imaging Array for Lens-less FLIM.
Lee, Changhyuk; Johnson, Ben; Jung, TaeSung; Molnar, Alyosha
2016-09-02
We present a 72 × 60, angle-sensitive single photon avalanche diode (A-SPAD) array for lens-less 3D fluorescence lifetime imaging. An A-SPAD pixel consists of (1) a SPAD to provide precise photon arrival time where a time-resolved operation is utilized to avoid stimulus-induced saturation, and (2) integrated diffraction gratings on top of the SPAD to extract incident angles of the incoming light. The combination enables mapping of fluorescent sources with different lifetimes in 3D space down to micrometer scale. Futhermore, the chip presented herein integrates pixel-level counters to reduce output data-rate and to enable a precise timing control. The array is implemented in standard 180 nm complementary metal-oxide-semiconductor (CMOS) technology and characterized without any post-processing.
A 72 × 60 Angle-Sensitive SPAD Imaging Array for Lens-less FLIM
Lee, Changhyuk; Johnson, Ben; Jung, TaeSung; Molnar, Alyosha
2016-01-01
We present a 72 × 60, angle-sensitive single photon avalanche diode (A-SPAD) array for lens-less 3D fluorescence lifetime imaging. An A-SPAD pixel consists of (1) a SPAD to provide precise photon arrival time where a time-resolved operation is utilized to avoid stimulus-induced saturation, and (2) integrated diffraction gratings on top of the SPAD to extract incident angles of the incoming light. The combination enables mapping of fluorescent sources with different lifetimes in 3D space down to micrometer scale. Futhermore, the chip presented herein integrates pixel-level counters to reduce output data-rate and to enable a precise timing control. The array is implemented in standard 180 nm complementary metal-oxide-semiconductor (CMOS) technology and characterized without any post-processing. PMID:27598170
Autoionizing resonances in electron-impact ionization of O5+ ions
NASA Astrophysics Data System (ADS)
Müller, A.; Teng, H.; Hofmann, G.; Phaneuf, R. A.; Salzborn, E.
2000-12-01
We report on a detailed experimental and theoretical study of electron-impact ionization of O5+ ions. A high-resolution scan measurement of the K-shell excitation threshold region has been performed with statistical uncertainties as low as 0.03%. At this level of precision a wealth of features in the cross section arising from indirect ionization processes becomes visible, and even interference of direct ionization with resonant-excitation/auto-double-ionization (READI) is clearly observed. The experimental results are compared with R-matrix calculations that include both direct and indirect processes in a unified way. Radiative damping of autoionizing Li-like states is found to be about 10-15 %. The calculations almost perfectly reproduce most of the experimental resonance features found in the present measurement including READI. They also agree with the direct-ionization converged close-coupling results of I. Bray [J. Phys. B 28, L247 (1995)] and the absolute total ionization cross section measurement of K. Rinn et al. [Phys. Rev. A 36, 595 (1987)].
Zhang, Peng; Lee, Seungah; Yu, Hyunung; ...
2015-06-15
Super-resolution imaging of fluorescence-free plasmonic nanoparticles (NPs) was achieved using enhanced dark-field (EDF) illumination based on wavelength-modulation. Indistinguishable adjacent EDF images of 103-nm gold nanoparticles (GNPs), 40-nm gold nanorods (GNRs), and 80-nm silver nanoparticles (SNPs) were modulated at their wavelengths of specific localized surface plasmon scattering. The coordinates (x, y) of each NP were resolved by fitting their point spread functions with a two-dimensional Gaussian. The measured localization precisions of GNPs, GNRs, and SNPs were 2.5 nm, 5.0 nm, and 2.9 nm, respectively. From the resolved coordinates of NPs and the corresponding localization precisions, super-resolution images were reconstructed. Depending onmore » the spontaneous polarization of GNR scattering, the orientation angle of GNRs in two-dimensions was resolved and provided more elaborate localization information. This novel fluorescence-free super-resolution method was applied to live HeLa cells to resolve NPs and provided remarkable subdiffraction limit images.« less
Non-contact measurement of rotation angle with solo camera
NASA Astrophysics Data System (ADS)
Gan, Xiaochuan; Sun, Anbin; Ye, Xin; Ma, Liqun
2015-02-01
For the purpose to measure a rotation angle around the axis of an object, a non-contact rotation angle measurement method based on solo camera was promoted. The intrinsic parameters of camera were calibrated using chessboard on principle of plane calibration theory. The translation matrix and rotation matrix between the object coordinate and the camera coordinate were calculated according to the relationship between the corners' position on object and their coordinates on image. Then the rotation angle between the measured object and the camera could be resolved from the rotation matrix. A precise angle dividing table (PADT) was chosen as the reference to verify the angle measurement error of this method. Test results indicated that the rotation angle measurement error of this method did not exceed +/- 0.01 degree.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Fujii, M.; Sato, K.; Kimura, K.
Photoelectron spectra due to autoionization for two series of high Rydberg states have been observed for diazabicyclooctane (DABCO) in a supersonic jet. The selection rule of the autoionization has been found to be ..delta..v = -1 for each vibrational mode involved in the Rydberg states, consistent with Berry's theory available for the vibrational autoionization of a polyatomic molecule. The relative autoionization efficiencies Phi/sub a/ for the high Rydberg series have also been determined from two-color MPI and fluorescence dip spectra. The irregular variation of Phi/sub a/ with the principal quantum number n has been found for the two Rydberg series,more » suggesting the irregular variation in their nonradiative rates« less
Autoionization structure of nitric oxide (NO) at the first ionization limit
DOE Office of Scientific and Technical Information (OSTI.GOV)
Miescher, E.; Lee, Y.T.; Guertler, P.
1978-03-15
A new and more detailed interpretation is given to the fine structure in the photoionization curve of cold NO observed by Ng, Mahan, and Lee. Resonances are assigned to autoionizing np and nddelta Rydberg levels which give prominent diffuse absorption bands in a spectrum recorded with the synchrotron radiation continuum. ..delta nu..<-1transitions in the vibrational autoionization process are substantiated.
The energy structure and decay channels of the 4p6-shell excited states in Sr
NASA Astrophysics Data System (ADS)
Kupliauskienė, A.; Kerevičius, G.; Borovik, V.; Shafranyosh, I.; Borovik, A.
2017-11-01
The ejected-electron spectra arising from the decay of the 4p{}5{{nln}}{\\prime }{l}{\\prime }{n}{\\prime\\prime }{l}{\\prime\\prime } autoionizing states in Sr atoms have been studied precisely at the incident-electron energies close to excitation and ionization thresholds of the 4{{{p}}}6 subshell. The excitation behaviors for 58 lines observed between 12 and 21 eV ejected-electron kinetic energy have been investigated. Also, the ab initio calculations of excitation energies, autoionization probabilities and electron-impact excitation cross sections of the states 4p{}5{{nln}}{\\prime }{l}{\\prime }{n}{\\prime\\prime }{l}{\\prime\\prime } (nl = 4d, 5s, 5p; {n}{\\prime }{l}{\\prime } = 4d, 5s, 5p; {n}{\\prime\\prime }{l}{\\prime\\prime } = 5s, 6s, 7s, 8s, 9s, 5p, 6p, 5d, 6d, 7d, 8d, 4f, 5g) have been performed by employing the large-scale configuration-interaction method in the basis of the solutions of Dirac-Fock-Slater equations. The obtained experimental and theoretical data have been used for the accurate identification of the 60 lines in ejected-electron spectra and the 68 lines observed earlier in photoabsorption spectra. The excitation and decay processes for 105 classified states in the 4p55s{}2{nl}, 4p54d{}2{nl} and 4p55s{{nln}}{\\prime }{l}{\\prime } configurations have been considered in detail. In particular, most of the states lying below the ionization threshold of the 4p6 subshell at 26.92 eV possess up to four decay channels with formation of Sr+ in 5s{}1/2, 4d{}3/{2,5/2} and 5p{}1/{2,3/2} states. Two-step autoionization and two-electron Auger transitions with formation of Sr2+ in the 4p6 {}1{{{S}}}0 ground state are the main decay paths for high-lying autoionizing states. The excitation threshold of the 4{{{p}}}6 subshell in Sr has been established at 20.98 ± 0.05 eV.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Doughty, Benjamin; Haber, Louis H.; Leone, Stephen R.
2011-10-15
Pump-probe photoelectron velocity-map imaging, using 27-eV high-harmonic excitation and 786-nm ionization, is used to resolve overlapping autoionizing resonances in atomic krypton, obtaining two-photon photoelectron angular distributions (PADs) for singly and doubly excited states. Two features in the photoelectron spectrum are assigned to singly excited 4s{sup 1}4p{sup 6}np{sup 1} (n = 7,8) configurations and four features provide information about double excitation configurations. The anisotropy parameters for the singly excited 7p configuration are measured to be {beta}{sub 2} = 1.61 {+-} 0.06 and {beta}{sub 4} = 1.54 {+-} 0.16 while the 8p configuration gives {beta}{sub 2} = 1.23 {+-} 0.19 and {beta}{submore » 4} = 0.60 {+-} 0.15. These anisotropies most likely represent the sum of overlapping PADs from states of singlet and triplet spin multiplicities. Of the four bands corresponding to ionization of doubly excited states, two are assigned to 4s{sup 2}4p{sup 4}5s{sup 1}6p{sup 1} configurations that are probed to different J-split ion states. The two remaining doubly excited states are attributed to a previously observed, but unassigned, resonance in the vacuum-ultraviolet photoabsorption spectrum. The PADs from each of the double excitation states are also influenced by overlap from neighboring states that are not completely spectrally resolved. The anisotropies of the observed double excitation states are reported, anticipating future theoretical and experimental work to separate the overlapping PADs into the state resolved PADs. The results can be used to test theories of excited state ionization.« less
Ambiguity Resolution for Phase-Based 3-D Source Localization under Fixed Uniform Circular Array.
Chen, Xin; Liu, Zhen; Wei, Xizhang
2017-05-11
Under fixed uniform circular array (UCA), 3-D parameter estimation of a source whose half-wavelength is smaller than the array aperture would suffer from a serious phase ambiguity problem, which also appears in a recently proposed phase-based algorithm. In this paper, by using the centro-symmetry of UCA with an even number of sensors, the source's angles and range can be decoupled and a novel algorithm named subarray grouping and ambiguity searching (SGAS) is addressed to resolve angle ambiguity. In the SGAS algorithm, each subarray formed by two couples of centro-symmetry sensors can obtain a batch of results under different ambiguities, and by searching the nearest value among subarrays, which is always corresponding to correct ambiguity, rough angle estimation with no ambiguity is realized. Then, the unambiguous angles are employed to resolve phase ambiguity in a phase-based 3-D parameter estimation algorithm, and the source's range, as well as more precise angles, can be achieved. Moreover, to improve the practical performance of SGAS, the optimal structure of subarrays and subarray selection criteria are further investigated. Simulation results demonstrate the satisfying performance of the proposed method in 3-D source localization.
NASA Astrophysics Data System (ADS)
Wang, Jing-Rong; Liu, Guo-Zhu; Zhang, Chang-Jin
2016-07-01
Angle-resolved upper critical field Hc 2 provides an efficient tool to probe the gap symmetry of unconventional superconductors. We revisit the behavior of in-plane Hc 2 in d -wave superconductors by considering both the orbital effect and Pauli paramagnetic effect. After carrying out systematic analysis, we show that the maxima of Hc 2 could be along either nodal or antinodal directions of a d -wave superconducting gap, depending on the specific values of a number of tuning parameters. This behavior is in contrast to the common belief that the maxima of in-plane Hc 2 are along the direction where the superconducting gap takes its maximal value. Therefore, identifying the precise d -wave gap symmetry through fitting experiments results of angle-resolved Hc 2 with model calculations at a fixed temperature, as widely used in previous studies, is difficult and practically unreliable. However, our extensive analysis of angle-resolved Hc 2 show that there is a critical temperature T*: in-plane Hc 2 exhibits its maxima along nodal directions at T
Full-Circle Resolver-to-Linear-Analog Converter
NASA Technical Reports Server (NTRS)
Alhorn, Dean C.; Smith, Dennis A.; Howard, David E.
2005-01-01
A circuit generates sinusoidal excitation signals for a shaft-angle resolver and, like the arctangent circuit described in the preceding article, generates an analog voltage proportional to the shaft angle. The disadvantages of the circuit described in the preceding article arise from the fact that it must be made from precise analog subcircuits, including a functional block capable of implementing some trigonometric identities; this circuitry tends to be expensive, sensitive to noise, and susceptible to errors caused by temperature-induced drifts and imprecise matching of gains and phases. These disadvantages are overcome by the design of the present circuit. The present circuit (see figure) includes an excitation circuit, which generates signals Ksin(Omega(t)) and Kcos(Omega(t)) [where K is an amplitude, Omega denotes 2(pi)x a carrier frequency (the design value of which is 10 kHz), and t denotes time]. These signals are applied to the excitation terminals of a shaft-angle resolver, causing the resolver to put out signals C sin(Omega(t)-Theta) and C cos(Omega(t)-Theta). The cosine excitation signal and the cosine resolver output signal are processed through inverting comparator circuits, which are configured to function as inverting squarers, to obtain logic-level or square-wave signals .-LL[cos(Omega(t)] and -LL[cos(Omega(t)-Theta)], respectively. These signals are fed as inputs to a block containing digital logic circuits that effectively measure the phase difference (which equals Theta between the two logic-level signals). The output of this block is a pulse-width-modulated signal, PWM(Theta), the time-averaged value of which ranges from 0 to 5 VDC as Theta ranges from .180 to +180deg. PWM(Theta) is fed to a block of amplifying and level-shifting circuitry, which converts the input PWM waveform to an output waveform that switches between precise reference voltage levels of +10 and -10 V. This waveform is processed by a two-pole, low-pass filter, which removes the carrier-frequency component. The final output signal is a DC potential, proportional to Theta that ranges continuously from -10 V at Theta = -180deg to +10 V at Theta = +180deg..
FLEET Velocimetry Measurements on a Transonic Airfoil
NASA Technical Reports Server (NTRS)
Burns, Ross A.; Danehy, Paul M.
2017-01-01
Femtosecond laser electronic excitation tagging (FLEET) velocimetry was used to study the flowfield around a symmetric, transonic airfoil in the NASA Langley 0.3-m TCT facility. A nominal Mach number of 0.85 was investigated with a total pressure of 125 kPa and total temperature of 280 K. Two-components of velocity were measured along vertical profiles at different locations above, below, and aft of the airfoil at angles of attack of 0 deg, 3.5 deg, and 7deg. Measurements were assessed for their accuracy, precision, dynamic range, spatial resolution, and overall measurement uncertainty in the context of the applied flowfield. Measurement precisions as low as 1 m/s were observed, while overall uncertainties ranged from 4 to 5 percent. Velocity profiles within the wake showed sufficient accuracy, precision, and sensitivity to resolve both the mean and fluctuating velocities and general flow physics such as shear layer growth. Evidence of flow separation is found at high angles of attack.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Bhaskaran-Nair, Kiran; Valiev, Marat; Deng, Shihu
2015-12-14
The photophysics of Green Fluorescent Protein (GFP) chromophore is critically dependent on its local structure and on its environment. Despite extensive experimental and computational studies, there remain many open questions regarding the key fundamental variables that govern this process. One outstanding problem is the role of autoionization as a possible relaxation pathway of the excited state under different environmental conditions. This issue is considered in our work through combined experimental and theoretical studies of microsolvated clusters of the deprotonated p-hydroxybenzylidene-2,3-dimethylimidazolinone anion (HBDI⁻), an analog of GFP chromophore. Through selective generation of microsolvated structures of predetermined size and subsequent analysis ofmore » experimental photoelectron spectra by high level ab-initio methods we are able to precisely identify the structure of the system, establish the accuracy of theoretical data, and provide reliable description of auto-ionization process as a function of hydrogen-bonding environment. Our study clearly illustrates the first few water molecules progressively stabilize the excited state of the chromophore anion against the autodetached neutral state, which should be an important trait for crystallographic water molecules in GFPs that has not been fully explored to date.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Bhaskaran-Nair, Kiran; Shelton, William A.; Center for Computation and Technology, Louisiana State University, Baton Rouge, Louisiana 70803
2015-12-14
The photophysics of the Green Fluorescent Protein (GFP) chromophore is critically dependent on its local structure and on its environment. Despite extensive experimental and computational studies, there remain many open questions regarding the key fundamental variables that govern this process. One outstanding problem is the role of autoionization as a possible relaxation pathway of the excited state under different environmental conditions. This issue is considered in our work through combined experimental and theoretical studies of microsolvated clusters of the deprotonated p-hydroxybenzylidene-2,3-dimethylimidazolinone anion (HBDI{sup −}), an analog of the GFP chromophore. Through selective generation of microsolvated structures of predetermined size andmore » subsequent analysis of experimental photoelectron spectra by high level ab initio methods, we are able to precisely identify the structure of the system, establish the accuracy of theoretical data, and provide reliable description of auto-ionization process as a function of hydrogen-bonding environment. Our study clearly illustrates the first few water molecules progressively stabilize the excited state of the chromophore anion against the autodetached neutral state, which should be an important trait for crystallographic water molecules in GFPs that has not been fully explored to date.« less
Electron Emission in Highly Charged Ion-Atom Collisions
NASA Astrophysics Data System (ADS)
Liao, Chunlei
1995-01-01
This dissertation addresses the problem of electron emission in highly charged ion-atom collisions. The study is carried out by measuring doubly differential cross sections (DDCS) of emitted electrons for projectiles ranging from fluorine up to gold at ejection angles (theta _{L}) from 0^circ to 70^circ with respect to the beam direction. Prominent features are a very strong forward peaked angular distribution of emitted electrons and the appearance of strong diffraction structures in the binary encounter electron (BEe) region for projectiles heavier than chlorine. This is in clear contradiction to the results found with fluorine projectiles, where the BEe production increases slightly with increasing theta_{L} and no structure is observed in the BEe region. Both can be understood in the impulse approximation as elastic scattering of quasi free target electrons in the projectile potential. Our measurements also show that the violation of q ^2 scaling of the DDCS previously established for 0^circ electron spectra persists for all emission angles and almost all electron energies. In ion-atom collisions, besides electrons from target, electrons from projectile ionization are also presented in the emitted electron spectra. Using electron-projectile coincidence technique, different collision channels can be separated. In order to eliminate the speculations of contributions from projectile related capture and loss channels, coincidence studies of diffraction structures are initiated. In the 0^circ electron spectrum of 0.3 MeV/u I^{6+} impacting on H_2, strong autoionization peaks are observed on the shoulders of the cusp peak. The energies of these autoionization lines in the projectile rest frame are determined by high-resolution electron spectroscopy, and collision mechanism is probed by electron-charge state selected projectile coincidence technique.
Nanoscale cellular imaging with scanning angle interference microscopy.
DuFort, Christopher; Paszek, Matthew
2014-01-01
Fluorescence microscopy is among the most widely utilized tools in cell and molecular biology due to its ability to noninvasively obtain time-resolved images of live cells with molecule-specific contrast. In this chapter, we describe a simple high-resolution technique, scanning angle interference microscopy (SAIM), for the imaging and localization of fluorescent molecules with nanometer precision along the optical axis. In SAIM, samples above a reflective surface are sequentially scanned with an excitation laser at varying angles of incidence. Interference patterns generated between the incident and reflected lights result in an emission intensity that depends on the height of a fluorophore above the silicon surface and the angle of the incident radiation. The measured fluorescence intensities are then fit to an optical model to localize the labeled molecules along the z-axis with 5-10 nm precision and diffraction-limited lateral resolution. SAIM is easily implemented on widely available commercial total internal reflection fluorescence microscopes, offering potential for widespread use in cell biology. Here, we describe the setup of SAIM and its application for imaging cellular structures near (<1 μm) the sample substrate. © 2014 Elsevier Inc. All rights reserved.
Cheaper Synthesis Of Multipole-Brushless-dc-Motor Current
NASA Technical Reports Server (NTRS)
Alhorn, Dean C.; Howard, David E.
1994-01-01
Circuit converts output of single two-phase shaft-angle resolver to that of multi-speed three-phase shaft-angle resolver. Converter circuit applicable to generation of multispeed, multiphase shaft-angle-resolver signals from single two-phase shaft-angle resolver. Combination of converter circuit and single two-phase shaft-angle resolver offer advantages in cost, weight, size, and complexity. Design readily adaptable to two-phase motor.
NASA Astrophysics Data System (ADS)
Wang, He
The few-cycle femtosecond laser pulse has proved itself to be a powerful tool for controlling the electron dynamics inside atoms and molecules. By applying such few-cycle pulses as a driving field, single isolated attosecond pulses can be produced through the high-order harmonic generation process, which provide a novel tool for capturing the real time electron motion. The first part of the thesis is devoted to the state of the art few-cycle near infrared (NIR) laser pulse development, which includes absolute phase control (carrier-envelope phase stabilization), amplitude control (power stabilization), and relative phase control (pulse compression and shaping). Then the double optical gating (DOG) method for generating single attosecond pulses and the attosecond streaking experiment for characterizing such pulses are presented. Various experimental limitations in the attosecond streaking measurement are illustrated through simulation. Finally by using the single attosecond pulses generated by DOG, an attosecond transient absorption experiment is performed to study the autoionization process of argon. When the delay between a few-cycle NIR pulse and a single attosecond XUV pulse is scanned, the Fano resonance shapes of the argon autoionizing states are modified by the NIR pulse, which shows the direct observation and control of electron-electron correlation in the temporal domain.
Photoionization studies with molecular beams
DOE Office of Scientific and Technical Information (OSTI.GOV)
Ng, C.Y.
1976-09-01
A molecular beam photoionization apparatus which combines the advantages of both the molecular beam method with photoionization mass spectrometry has been designed and constructed for carrying out some unique photoionization experiments. Rotational cooling during the supersonic expansion has resulted in high resolution photoionization efficiency curves for NO, ICl, C/sub 2/H/sub 2/ and CH/sub 3/I. The analysis of these spectra has yielded ionization potentials for these molecules to an accuracy of +- 3 MeV. Detailed autoionization structures were also resolved. This allows the investigation of the selection rules for autoionization, and the identification of the Rydberg series which converge to themore » excited states of the molecular ions. The degree of relaxation for thermally populated excited states has been examined using NO and ICl as examples. As a result of adiabatic cooling, a small percentage of dimers is also formed during the expansion. The photoionization efficiency curves for (NO)/sub 2/, ArICl, Ar/sub 2/, Kr/sub 2/ and Xe/sub 2/ have been obtained near the thresholds. Using the known dissociation energies of the (NO)/sub 2/, Ar/sub 2/, Kr/sub 2/ and Xe/sub 2/ van der Waals molecules, the corresponding dissociation energies for NO-NO/sup +/, Ar/sub 2//sup +/, Kr/sub 2//sup +/, and Xe/sub 2//sup +/ have been determined. The ionization mechanisms for this class of molecules are examined and discussed.« less
Tachometer Derived From Brushless Shaft-Angle Resolver
NASA Technical Reports Server (NTRS)
Howard, David E.; Smith, Dennis A.
1995-01-01
Tachometer circuit operates in conjunction with brushless shaft-angle resolver. By performing sequence of straightforward mathematical operations on resolver signals and utilizing simple trigonometric identity, generates voltage proportional to rate of rotation of shaft. One advantage is use of brushless shaft-angle resolver as main source of rate signal: no brushes to wear out, no brush noise, and brushless resolvers have proven robustness. No switching of signals to generate noise. Another advantage, shaft-angle resolver used as shaft-angle sensor, tachometer input obtained without adding another sensor. Present circuit reduces overall size, weight, and cost of tachometer.
Control of the seven-degree-of-freedom upper limb exoskeleton for an improved human-robot interface
NASA Astrophysics Data System (ADS)
Kim, Hyunchul; Kim, Jungsuk
2017-04-01
This study analyzes a practical scheme for controlling an exoskeleton robot with seven degrees of freedom (DOFs) that supports natural movements of the human arm. A redundant upper limb exoskeleton robot with seven DOFs is mechanically coupled to the human body such that it becomes a natural extension of the body. If the exoskeleton robot follows the movement of the human body synchronously, the energy exchange between the human and the robot will be reduced significantly. In order to achieve this, the redundancy of the human arm, which is represented by the swivel angle, should be resolved using appropriate constraints and applied to the robot. In a redundant 7-DOF upper limb exoskeleton, the pseudoinverse of the Jacobian with secondary objective functions is widely used to resolve the redundancy that defines the desired joint angles. A secondary objective function requires the desired joint angles for the movement of the human arm, and the angles are estimated by maximizing the projection of the longest principle axis of the manipulability ellipsoid for the human arm onto the virtual destination toward the head region. Then, they are fed into the muscle model with a relative damping to achieve more realistic robot-arm movements. Various natural arm movements are recorded using a motion capture system, and the actual swivel-angle is compared to that estimated using the proposed swivel angle estimation algorithm. The results indicate that the proposed algorithm provides a precise reference for estimating the desired joint angle with an error less than 5°.
Infrared studies of autoionization of thin films of dinitrogen tetroxidea)
NASA Astrophysics Data System (ADS)
Jones, L. H.; Swanson, B. I.; Agnew, S. F.
1985-05-01
The autoionization of dinitrogen tetroxide to form nitrosonium nitrate in thin films at 150-200 K has been studied using infrared absorption spectroscopy. It is found that at these temperatures and low pressure the process is intramolecular, involving only one of two isomers of the nitrite form (ONONO2). (AIP)
[Optics heterodyne detection of the autoionization state of barium].
Sun, Jiang; Su, Hong-xin; Wang, Yan-bang; Guo, Qing-lin; Zuo, Zhan-chun; Fu, Pan-ming
2008-06-01
The autoionization state of barium was observed by optics heterodyne between three-photon resonant nondegenerated six-wave mixing (NSWM) and two-photon resonant nondegenerated four-wave mixing (NFWM). In this way, optics heterodyne spectrum of 6p(3/2) 19d autoionization state of barium was measured. The suppression and enhancement of the NFWM signal was observed which was caused by the quantum interference between NFWM and NSWM. Our method is a pure nonlinear optic technique. It has the advantages of excellent spatial signal resolution and simple optical alignment. Here two-photon resonant NFWM is used as local oscillation, while three-photon resonant NSWM signal is used as signal beam. Detection of autoionization states of Ba was achieved by changing the frequency of signal beam. The phase matching condition of this technique is not so stringent and can be achieved over a very wide frequency range, which is very difficult in the general six-wave mixing. Furthermore, the signal is coherent light. Optics heterodyne spectrum is a Doppler-free spectroscopy when the incident lasers have narrow bandwidths.
Photoelectron imaging of autoionizing states of xenon: Effect of external electric fields
DOE Office of Scientific and Technical Information (OSTI.GOV)
Shubert, V. Alvin; Pratt, Stephen T.
Velocity map photoelectron imaging was used to study the photoelectron angular distributions of autoionizing Stark states of atomic xenon excited just below the Xe{sup +} {sup 2} P{sub 1/2}{sup o} threshold at fields ranging from 50 to 700 V/cm. Two-color, two-photon resonant, three-photon excitation via the 6p{sup '}[1/2]{sub 0} level was used to probe the region of interest. The wavelength scans show a similar evolution of structure to that observed in single-photon excitation [Ernst et al., Phys. Rev. A 37, 4172 (1988)]. The photoelectron angular distributions following autoionization of the Stark states provide information on the decay of excited statesmore » in electron fields. In the present experiments, the large autoionization width of the ({sup 2} P{sub 1/2}{sup o})nd[3/2]{sub 1}{sup o} series dominates the decay processes, and thus controls the angular distributions. However, the angular distributions of the Stark states also indicate the presence of other decay channels contributing to the decay of these states.« less
Ju, Sailong; Bai, Wei; Wu, Liming; Lin, Hua; Xiao, Chong; Cui, Shengtao; Li, Zhou; Kong, Shuai; Liu, Yi; Liu, Dayong; Zhang, Guobin; Sun, Zhe; Xie, Yi
2018-01-01
The ability to accurately determine the electronic structure of solids has become a key prerequisite for modern functional materials. For example, the precise determination of the electronic structure helps to balance the three thermoelectric parameters, which is the biggest challenge to design high-performance thermoelectric materials. Herein, by high-resolution, angle-resolved photoemission spectroscopy (ARPES), the itinerant carriers in CsBi 4 Te 6 (CBT) are revealed for the first time. CBT is a typical anisotropic, narrow-gap semiconductor used as a practical candidate for low-temperature thermoelectric applications, and p-doped CBT series show superconductivity at relatively low carrier concentrations. The ARPES results show a significantly larger bandwidth near the Fermi surface than calculations, which means the carriers transport anisotropically and itinerantly in CBT. It is reasonable to believe that these newly discovered features of carriers in narrow-gap semiconductors are promising for designing optimal thermoelectric materials and superconductors. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Forces on nuclei moving on autoionizing molecular potential energy surfaces.
Moiseyev, Nimrod
2017-01-14
Autoionization of molecular systems occurs in diatomic molecules and in small biochemical systems. Quantum chemistry packages enable calculation of complex potential energy surfaces (CPESs). The imaginary part of the CPES is associated with the autoionization decay rate, which is a function of the molecular structure. Molecular dynamics simulations, within the framework of the Born-Oppenheimer approximation, require the definition of a force field. The ability to calculate the forces on the nuclei in bio-systems when autoionization takes place seems to rely on an understanding of radiative damages in RNA and DNA arising from the release of slow moving electrons which have long de Broglie wavelengths. This work addresses calculation of the real forces on the nuclei moving on the CPES. By using the transformation of the time-dependent Schrödinger equation, previously used by Madelung, we proved that the classical forces on nuclei moving on the CPES correlated with the gradient of the real part of the CPES. It was proved that the force on the nuclei of the metastable molecules is time independent although the probability to detect metastable molecules exponentially decays. The classical force is obtained from the transformed Schrödinger equation when ℏ=0 and the Schrödinger equation is reduced to the classical (Newtonian) equations of motion. The forces on the nuclei regardless on what potential energy surface they move (parent CPES or product real PESs) vary in time due to the autoionization process.
NASA Technical Reports Server (NTRS)
Finkenthal, M.; Littman, A.; Stutman, D.; Bhatia, A. K.
1989-01-01
Spectra emitted by Al II and Al III in the 100-1900-A range from a Penning ionization discharge (PID) have been analyzed in order to study the populating mechanisms of the autoionizing levels of the Al III ion. Electron temperature and density estimates and Al III line intensities obtained using a collisional-radiative model are found to differ from those obtained experimentally, implying that the autoionizing levels of the Na I-like ion may be populated, in the PID plasma, by the inner-shell ionization of excited Mg I-like ions. It is suggested that such autoionizing lines could be used to search for populations inversions in the soft X-ray domain.
NASA Astrophysics Data System (ADS)
Ward, R.; Cubric, D.; Bowring, N.; King, G. C.; Read, F. H.; Fursa, D. V.; Bray, I.
2013-02-01
Excitation function measurements for the decay of the 2s22p 2P and 2s2p2 2D triply excited negative ion resonances in helium to singly excited n = 2 states have been measured. These excitation functions have been determined across the complete angular range (0-180°) using a magnetic angle changer with a soft-iron core. The convergent close-coupling method has been used to calculate the cross sections, with the underlying complexity of the problem not yet being able to be fully resolved. Agreement between the present experimental data and previous experimental data is good, with these excitation functions confirming the presence of an unusual (2s22p)2P resonance behaviour in the 21S channel at 90°, where this would not usually be expected. Resonance energy and width values have been obtained, with a mean energy for the (2s22p)2P resonance of 57.20 ± 0.08 eV and a mean width of 73 ± 20 meV, and a mean energy of the (2s2p2)2D resonance of 58.30 ± 0.08 eV and a mean width of 59 ± 27 meV. Resonant cross section and ρ2 values have been calculated across the angular range for the first time, providing angular distribution data on decay propensities for both resonances.
''Reading'' the photoelectron {beta}-parameter spectrum in a resonance region
DOE Office of Scientific and Technical Information (OSTI.GOV)
Dolmatov, V. K.; Guler, E.; Manson, S. T.
2007-09-15
The behavior of the dipole photoelectron angular distribution parameter {beta}{sub nl}({omega}) in the vicinity of autoionizing resonances is discussed. It is shown that from this behavior, surprisingly, many photoionization parameters that cannot be measured experimentally can be extracted. These are the energy positions and ordering of autoionizing resonance minima in the partial photoionization cross sections {sigma}{sub l+1} and {sigma}{sub l-1}, the energies at which these two cross sections intersect, and signs and magnitudes of the cos({delta}{sub l+1}-{delta}{sub l-1}) ({delta}{sub l{+-}}{sub 1} being the phase shifts of the dipole photoionization amplitudes D{sub l{+-}}{sub 1}, respectively) through the autoionizing resonance energy region.more » Based on this, a deeper interpretation of such effects as the width-narrowing, width-fluctuating, and q-reversal in the {beta}{sub nl} parameter spectrum in the autoionizing resonance energy region is given. As an example, calculated data for partial photoionization cross sections {sigma}{sub 3d{r_reversible}}{sub f} and {sigma}{sub 3d{r_reversible}}{sub p}, and {beta}{sub 3d} parameters for 3d photoelectrons from Cr{sup +} are presented.« less
Autoionization following nanoplasma formation in atomic and molecular clusters
NASA Astrophysics Data System (ADS)
Schütte, Bernd; Lahl, Jan; Oelze, Tim; Krikunova, Maria; Vrakking, Marc J. J.; Rouzée, Arnaud
2016-05-01
Nanoplasmas resulting from the ionization of nano-scale particles by intense laser pulses are typically described by quasiclassical models, where electron emission is understood to take place via thermal processes. Recently, we discovered that, following the interaction of intense near-infrared (NIR) laser pulses with molecular oxygen clusters, electron emission from nanoplasmas can also occur from atomic bound states via autoionization [Schütte et al., Phys. Rev. Lett. 114, 123002 (2015)]. Here we extend these studies and demonstrate that the formation and decay of doubly-excited atoms and ions is a very common phenomenon in nanoplasmas. We report on the observation of autoionization involving spin-orbit excited states in molecular oxygen and carbon dioxide clusters as well as in atomic krypton and xenon clusters ionized by intense NIR pulses, for which we find clear bound-state signatures in the electron kinetic energy spectra. By applying terahertz (THz) streaking, we show that the observed autoionization processes take place on a picosecond to nanosecond timescale after the interaction of the NIR laser pulse with the clusters. Contribution to the Topical Issue "Atomic Cluster Collisions (7th International Symposium)", edited by Gerardo Delgado Barrio, Andrey Solov'Yov, Pablo Villarreal, Rita Prosmiti.
Ultrafast laser control of autoionizing resonances observed in attosecond transient absorption
NASA Astrophysics Data System (ADS)
Liao, Chen-Ting; Harkema, Nathan; Sandhu, Arvinder
2017-04-01
Attosecond and femtosecond extreme ultraviolet (XUV) pulses can be used to probe electron dynamics in high-lying excited states that autoionize on a femtosecond timescale, thus providing information on the process of Auger decay and its interference with the continua. Here we utilize XUV pulses in connection with infrared (IR) pulses to perform attosecond transient absorption spectroscopy of the impulsive response of argon autoionizing Rydberg states in the vicinity of the 3s-1 4 p resonance. We show that by tuning the time delay and field polarization of IR pulse, it is possible to control the dipolar coupling between neighboring states and hence the spectral line shape of the resonance, such as the transition between Breit-Wigner to Beutler-Fano profiles. NSF Grant No. PHY-1505556.
D autoionization states of He and ionic H
NASA Technical Reports Server (NTRS)
Bhatia, A. K.
1972-01-01
Positions of the lowest 1,3De autoionization states of He and H(-) below the n = 2 level of the He(+) and H were calculated variationally, using Feshbach's Q-operator formalism. The trial wave function is of the Hylleraas-type with appropriate angular momentum factors. The widths and the shifts of the states have also been calculated. The shifts are found to be positive for all the states calculated here. The results with 112 terms for most states are lower than any previously calculated. The calculated lowest autoionization states of the He and H(-) (relative to the ground states of He and H respectively) are 59.902 eV and 10.1185 eV, in good agreement with the observed values of 59.9 eV and 10.13 + or 0.015 eV.
NASA Astrophysics Data System (ADS)
Zhou, Xingjiang; He, Shaolong; Liu, Guodong; Zhao, Lin; Yu, Li; Zhang, Wentao
2018-06-01
The significant progress in angle-resolved photoemission spectroscopy (ARPES) in last three decades has elevated it from a traditional band mapping tool to a precise probe of many-body interactions and dynamics of quasiparticles in complex quantum systems. The recent developments of deep ultraviolet (DUV, including ultraviolet and vacuum ultraviolet) laser-based ARPES have further pushed this technique to a new level. In this paper, we review some latest developments in DUV laser-based photoemission systems, including the super-high energy and momentum resolution ARPES, the spin-resolved ARPES, the time-of-flight ARPES, and the time-resolved ARPES. We also highlight some scientific applications in the study of electronic structure in unconventional superconductors and topological materials using these state-of-the-art DUV laser-based ARPES. Finally we provide our perspectives on the future directions in the development of laser-based photoemission systems.
Three-dimensional super-resolved live cell imaging through polarized multi-angle TIRF.
Zheng, Cheng; Zhao, Guangyuan; Liu, Wenjie; Chen, Youhua; Zhang, Zhimin; Jin, Luhong; Xu, Yingke; Kuang, Cuifang; Liu, Xu
2018-04-01
Measuring three-dimensional nanoscale cellular structures is challenging, especially when the structure is dynamic. Owing to the informative total internal reflection fluorescence (TIRF) imaging under varied illumination angles, multi-angle (MA) TIRF has been examined to offer a nanoscale axial and a subsecond temporal resolution. However, conventional MA-TIRF still performs badly in lateral resolution and fails to characterize the depth image in densely distributed regions. Here, we emphasize the lateral super-resolution in the MA-TIRF, exampled by simply introducing polarization modulation into the illumination procedure. Equipped with a sparsity and accelerated proximal algorithm, we examine a more precise 3D sample structure compared with previous methods, enabling live cell imaging with a temporal resolution of 2 s and recovering high-resolution mitochondria fission and fusion processes. We also shared the recovery program, which is the first open-source recovery code for MA-TIRF, to the best of our knowledge.
Narrow chaotic compound autoionizing states in atomic spectra
DOE Office of Scientific and Technical Information (OSTI.GOV)
Flambaum, V.V.; Gribakina, A.A.; Gribakin, G.F.
1996-09-01
Simultaneous excitation of several valence electrons in atoms gives rise to a dense spectrum of compound autoionizing states (AIS). These states are almost chaotic superpositions of large numbers of many-electron basis states built of single-electron orbitals. The mean level spacing {ital D} between such states is very small (e.g., {ital D}{lt}0.01 eV for the numerical example of {ital J}{sup {pi}}=4{sup {minus}} states of Ce just above the ionization threshold). The autoionization widths of these states estimated by perturbations, {gamma}=2{pi}{vert_bar}{ital W}{vert_bar}{sup 2}, where {ital W} is the Coulomb matrix element coupling the AIS to the continuum, are also small, but comparablemore » with {ital D} in magnitude: {gamma}{approximately}{ital D}. Hence the nonperturbative interaction of AIS with each other via the continuum is very essential. It suppresses greatly the widths of the autoionizing resonances ({Gamma}{approx_equal}{ital D}{sup 2}/3{gamma}{lt}{ital D}), and leads to the emergence of a {open_quote}{open_quote}collective{close_quote}{close_quote} doorway state which accumulates a large share of the total width. This state is in essence a modified single-particle continuum decoupled from the resonances due to its large width. Narrow compound AIS should be a common feature of atomic spectra at energies sufficient for excitation of several electrons above the ground-state configuration. The narrow resonances can be observed as peaks in the photoabsorption, or, in electron-ion scattering, as Fano-type profiles on the background provided by the wide doorway-state resonance. It is also shown that the statistics of electromagnetic and autoionization amplitudes involving compound states are close to Gaussian. {copyright} {ital 1996 The American Physical Society.}« less
NASA Technical Reports Server (NTRS)
Moore, E. N.; Altick, P. L.
1972-01-01
The research performed is briefly reviewed. A simple method was developed for the calculation of continuum states of atoms when autoionization is present. The method was employed to give the first theoretical cross section for beryllium and magnesium; the results indicate that the values used previously at threshold were sometimes seriously in error. These threshold values have potential applications in astrophysical abundance estimates.
A classification model of Hyperion image base on SAM combined decision tree
NASA Astrophysics Data System (ADS)
Wang, Zhenghai; Hu, Guangdao; Zhou, YongZhang; Liu, Xin
2009-10-01
Monitoring the Earth using imaging spectrometers has necessitated more accurate analyses and new applications to remote sensing. A very high dimensional input space requires an exponentially large amount of data to adequately and reliably represent the classes in that space. On the other hand, with increase in the input dimensionality the hypothesis space grows exponentially, which makes the classification performance highly unreliable. Traditional classification algorithms Classification of hyperspectral images is challenging. New algorithms have to be developed for hyperspectral data classification. The Spectral Angle Mapper (SAM) is a physically-based spectral classification that uses an ndimensional angle to match pixels to reference spectra. The algorithm determines the spectral similarity between two spectra by calculating the angle between the spectra, treating them as vectors in a space with dimensionality equal to the number of bands. The key and difficulty is that we should artificial defining the threshold of SAM. The classification precision depends on the rationality of the threshold of SAM. In order to resolve this problem, this paper proposes a new automatic classification model of remote sensing image using SAM combined with decision tree. It can automatic choose the appropriate threshold of SAM and improve the classify precision of SAM base on the analyze of field spectrum. The test area located in Heqing Yunnan was imaged by EO_1 Hyperion imaging spectrometer using 224 bands in visual and near infrared. The area included limestone areas, rock fields, soil and forests. The area was classified into four different vegetation and soil types. The results show that this method choose the appropriate threshold of SAM and eliminates the disturbance and influence of unwanted objects effectively, so as to improve the classification precision. Compared with the likelihood classification by field survey data, the classification precision of this model heightens 9.9%.
Sohn, Martin Y; Barnes, Bryan M; Silver, Richard M
2018-03-01
Accurate optics-based dimensional measurements of features sized well-below the diffraction limit require a thorough understanding of the illumination within the optical column and of the three-dimensional scattered fields that contain the information required for quantitative metrology. Scatterfield microscopy can pair simulations with angle-resolved tool characterization to improve agreement between the experiment and calculated libraries, yielding sub-nanometer parametric uncertainties. Optimized angle-resolved illumination requires bi-telecentric optics in which a telecentric sample plane defined by a Köhler illumination configuration and a telecentric conjugate back focal plane (CBFP) of the objective lens; scanning an aperture or an aperture source at the CBFP allows control of the illumination beam angle at the sample plane with minimal distortion. A bi-telecentric illumination optics have been designed enabling angle-resolved illumination for both aperture and source scanning modes while yielding low distortion and chief ray parallelism. The optimized design features a maximum chief ray angle at the CBFP of 0.002° and maximum wavefront deviations of less than 0.06 λ for angle-resolved illumination beams at the sample plane, holding promise for high quality angle-resolved illumination for improved measurements of deep-subwavelength structures using deep-ultraviolet light.
Two-photon spectroscopy of autoionizing states of Xe² near threshold
DOE Office of Scientific and Technical Information (OSTI.GOV)
Pratt, Stephen T.; Dehmer, Patricia M.; Dehmer, Joseph L.
1990-01-01
The two-photon ionization spectrum of Xe² in the region of the first ionization threshold is presented. Vibronic bands corresponding to at least four different autoionizing electronic states of Xe² are observed for the first time and are tentatively assigned. The observed appearance potential is significantly higher (by 415 cm-1) than the earlier single-photon ionization result (Ng, Trevor, Mahan and Lee, - J. Chem. Phys. 65 (1976) 4327).
Photoionization research on atomic beams. 2: The photoionization cross section of atomic oxygen
NASA Technical Reports Server (NTRS)
Comes, F. J.; Speier, F.; Elzer, A.
1982-01-01
An experiment to determine the absolute value of the photo-ionization cross section of atomic oxygen is described. The atoms are produced in an electrical discharge in oxygen gas with 1% hydrogen added. In order to prevent recombination a crossed beam technique is employed. The ions formed are detected by a time-of-flight mass spectrometer. The concentration of oxygen atoms in the beam is 57%. The measured photoionization cross section of atomic oxygen is compared with theoretical data. The results show the participation of autoionization processes in ionization. The cross section at the autoionizing levels detected is considerably higher than the absorption due to the unperturbed continuum. Except for wavelengths where autoionization occurs, the measured ionization cross section is in fair agreement with theory. This holds up to 550 A whereas for shorter wavelengths the theoretical values are much higher.
Photoionization and electron-impact ionization of Ar5+
DOE Office of Scientific and Technical Information (OSTI.GOV)
Wang, J.C.; Lu, M.; Esteves, D.
2007-02-27
Absolute cross sections for photoionization andelectron-impact Photionization of Ar5+ have been measuredusing twodifferent interacting-beams setups. The spectra consist of measurementsof the yield of products dueto single ionization as a function ofelectron or photon energy. In addition, absolute photoionization andelectron-impact ionization cross sections were measured to normalize themeasured Ar6+ product-ion yield spectra. In the energy range from 90 to111 eV, both electron-impact ionization and photoionization of Ar5+aredominated by indirect 3s subshell excitation-autoionization. In theenergy range from 270 to 285 eV, resonances due to 2p-3dexcitation-autoionization are prominent in the photoionization spectrum.In the range from 225 to 335 eV, an enhancement due tomore » 2p-nl (n>2>excitations are evident in the electron-impactionization cross section.The electron and photon impact data show some features due to excitationof the same intermediate autoionizing states.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
KETTELL, S.; ET AL.
2006-10-16
This document describes the design of the Daya Bay reactor neutrino experiment. Recent discoveries in neutrino physics have shown that the Standard Model of particle physics is incomplete. The observation of neutrino oscillations has unequivocally demonstrated that the masses of neutrinos are nonzero. The smallness of the neutrino masses (<2 eV) and the two surprisingly large mixing angles measured have thus far provided important clues and constraints to extensions of the Standard Model. The third mixing angle, {delta}{sub 13}, is small and has not yet been determined; the current experimental bound is sin{sup 2} 2{theta}{sub 13} < 0.17 at 90%more » confidence level (from Chooz) for {Delta}m{sub 31}{sup 2} = 2.5 x 10{sup -3} eV{sup 2}. It is important to measure this angle to provide further insight on how to extend the Standard Model. A precision measurement of sin{sup 2} 2{theta}{sub 13} using nuclear reactors has been recommended by the 2004 APS Multi-divisional Study on the Future of Neutrino Physics as well as a recent Neutrino Scientific Assessment Group (NUSAG) report. We propose to perform a precision measurement of this mixing angle by searching for the disappearance of electron antineutrinos from the nuclear reactor complex in Daya Bay, China. A reactor-based determination of sin{sup 2} 2{theta}{sub 13} will be vital in resolving the neutrino-mass hierarchy and future measurements of CP violation in the lepton sector because this technique cleanly separates {theta}{sub 13} from CP violation and effects of neutrino propagation in the earth. A reactor-based determination of sin{sup 2} 2{theta}{sub 13} will provide important, complementary information to that from long-baseline, accelerator-based experiments. The goal of the Daya Bay experiment is to reach a sensitivity of 0.01 or better in sin{sup 2} 2{theta}{sub 13} at 90% confidence level.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Behar, Ehud; Jacobs, Verne L.; Oreg, Joseph
Total cross sections for electron-ion photorecombination (PR) processes are calculated using a projection-operator and resolvent-operator approach. This approach provides a unified quantum-mechanical description of the combined electron-ion PR process, including radiative and dielectronic recombination as coherent, interfering components. An especially adapted version of the Hebrew-University Lawrence-Livermore Atomic Code HULLAC is developed and employed for the calculations. In particular, PR cross sections for He-like argon and iron ions are calculated for incident-electron energies in the vicinity of the 1s2l2l{sup '} and 1s2l3l{sup '} doubly-excited, autoionizing levels of the Li-like ions. Significant effects of quantum interference between radiative and dielectronic recombination, inmore » the form of asymmetric PR cross-section profiles, are predicted, especially for weak transitions. The general behavior of the interference effect, as a function of the ion charge q and as a function of the principal quantum number n{sup '} of the outer electron in the autoionizing state, is investigated using a hydrogenic-scaling analysis. It is found that the degree of asymmetry in the PR cross-section profile can be substantial for close-to-neutral ions and also for very highly-charged ions. In the intermediate-charge regime, on the other hand, the asymmetry is anticipated to be less prominent. The dependence of the quantum-interference effect on n{sup '} is predicted to be much weaker.« less
Research on the properties and interactions of simple atomic and ionic systems
NASA Technical Reports Server (NTRS)
Novick, R.
1972-01-01
Simple ionic systems were studied, such as metastable autoionizing states of the negative He ion, two-photon decay spectrum of metastable He ion, optical excitation with low energy ions, and lifetime measurements of singly ionized Li and metastable He ion. Simple atomic systems were also investigated. Metastable autoionizing atomic energy levels in alkali elements were included, along with lifetime measurements of Cr-53, group 2A isotopes, and alkali metal atoms using level crossing and optical double resonance spectroscopy.
NASA Astrophysics Data System (ADS)
Locht, R.; Leyh, B.; Dehareng, D.; Hottmann, K.; Baumgärtel, H.
2010-01-01
The threshold photoelectron spectrum (TPES) and the constant ion state (CIS) spectra of the individual ionic states of C2H3F have been recorded using synchrotron radiation. For comparison a well-resolved HeI photoelectron spectrum (HeI-PES) has also been measured and analysed in detail. The TPES has been measured between 9.5 eV and 35 eV photon energy. Numerous vibrational structures, reported for the first time, observed in the ground state and the six excited states of the cation are analysed. Quantum chemical calculations have been performed and provide strong support to the assignments. State-selected CIS spectra highlighted the major importance of autoionization for the production of almost all ionized states of C2H3F observed in this work.
NASA Astrophysics Data System (ADS)
Marmiroli, Benedetta; Grenci, Gianluca; Cacho-Nerin, Fernando; Sartori, Barbara; Laggner, Peter; Businaro, Luca; Amenitsch, Heinz
2010-02-01
Recently, we have designed, fabricated and tested a free-jet micromixer for time resolved small angle X-ray scattering (SAXS) studies of nanoparticles formation in the <100 μs time range. The microjet has a diameter of 25 μm and a time of first accessible measurement of 75 μs has been obtained. This result can still be improved. In this communication, we present a method to estimate whether a given chemical or biological reaction can be investigated with the micromixer, and to optimize the beam size for the measurement at the chosen SAXS beamline. Moreover, we describe a system based on stereoscopic imaging which allows the alignment of the jet with the X-ray beam with a precision of 20 μm. The proposed experimental procedures have been successfully employed to observe the formation of calcium carbonate (CaCO 3) nanoparticles from the reaction of sodium carbonate (Na 2CO 3) and calcium chloride (CaCl 2). The induction time has been estimated in the order of 200 μs and the determined radius of the particles is about 14 nm.
Spectral phase measurement of a Fano resonance using tunable attosecond pulses
Kotur, M.; Guénot, D.; Jiménez-Galán, Á; Kroon, D.; Larsen, E. W.; Louisy, M.; Bengtsson, S.; Miranda, M.; Mauritsson, J.; Arnold, C. L.; Canton, S. E.; Gisselbrecht, M.; Carette, T.; Dahlström, J. M.; Lindroth, E.; Maquet, A.; Argenti, L.; Martín, F.; L'Huillier, A.
2016-01-01
Electron dynamics induced by resonant absorption of light is of fundamental importance in nature and has been the subject of countless studies in many scientific areas. Above the ionization threshold of atomic or molecular systems, the presence of discrete states leads to autoionization, which is an interference between two quantum paths: direct ionization and excitation of the discrete state coupled to the continuum. Traditionally studied with synchrotron radiation, the probability for autoionization exhibits a universal Fano intensity profile as a function of excitation energy. However, without additional phase information, the full temporal dynamics cannot be recovered. Here we use tunable attosecond pulses combined with weak infrared radiation in an interferometric setup to measure not only the intensity but also the phase variation of the photoionization amplitude across an autoionization resonance in argon. The phase variation can be used as a fingerprint of the interactions between the discrete state and the ionization continua, indicating a new route towards monitoring electron correlations in time. PMID:26887682
NASA Astrophysics Data System (ADS)
Locke, Clayton R.; Kobayashi, Tohru; Midorikawa, Katsumi
2017-01-01
Odd-mass-selective ionization of palladium for purposes of resource recycling and management of long-lived fission products can be achieved by exploiting transition selection rules in a well-established three-step excitation process. In this conventional scheme, circularly polarized lasers of the same handedness excite isotopes via two intermediate 2D5/2 core states, and a third laser is then used for ionization via autoionizing Rydberg states. We propose an alternative excitation scheme via intermediate 2D3/2 core states before the autoionizing Rydberg state, improving ionization efficiency by over 130 times. We confirm high selectivity and measure odd-mass isotopes of >99.7(3)% of the total ionized product. We have identified and measured the relative ionization efficiency of the series of Rydberg states that converge to upper ionization limit of the 4 d 9(2D3/2) level, and identify the most efficient excitation is via the Rydberg state at 67668.18(10) cm-1.
Universal Long-Range Nanometric Bending of Water by Light.
Verma, Gopal; Singh, Kamal P
2015-10-02
Resolving mechanical effects of light on fluids has fundamental importance with wide applications. Most experiments to date on optofluidic interface deformation exploited radiation forces exerted by normally incident lasers. However, the intriguing effects of photon momentum for any configuration, including the unique total internal reflection regime, where an evanescent wave leaks above the interface, remain largely unexplored. A major difficulty in resolving nanomechanical effects has been the lack of a sensitive detection technique. Here, we devise a simple setup whereby a probe laser produces high-contrast Newton-ring-like fringes from a sessile water drop. The mechanical action of the photon momentum of a pump beam modulates the fringes, thus allowing us to perform a direct noninvasive measurement of a nanometric bulge with sub-5-nm precision. Remarkably, a <10 nm difference in the height of the bulge due to different laser polarizations and nonlinear enhancement in the bulge near total internal reflection is isolated. In addition, the nanometric bulge is shown to extend far longer, 100 times beyond the pump spot. Our high precision data validate the century-old Minkowski theory for a general angle and offer potential for novel optofluidic devices and noncontact nanomanipulation strategies.
A project based on multi-configuration Dirac-Fock calculations for plasma spectroscopy
NASA Astrophysics Data System (ADS)
Comet, M.; Pain, J.-C.; Gilleron, F.; Piron, R.
2017-09-01
We present a project dedicated to hot plasma spectroscopy based on a Multi-Configuration Dirac-Fock (MCDF) code, initially developed by J. Bruneau. The code is briefly described and the use of the transition state method for plasma spectroscopy is detailed. Then an opacity code for local-thermodynamic-equilibrium plasmas using MCDF data, named OPAMCDF, is presented. Transition arrays for which the number of lines is too large to be handled in a Detailed Line Accounting (DLA) calculation can be modeled within the Partially Resolved Transition Array method or using the Unresolved Transition Arrays formalism in jj-coupling. An improvement of the original Partially Resolved Transition Array method is presented which gives a better agreement with DLA computations. Comparisons with some absorption and emission experimental spectra are shown. Finally, the capability of the MCDF code to compute atomic data required for collisional-radiative modeling of plasma at non local thermodynamic equilibrium is illustrated. In addition to photoexcitation, this code can be used to calculate photoionization, electron impact excitation and ionization cross-sections as well as autoionization rates in the Distorted-Wave or Close Coupling approximations. Comparisons with cross-sections and rates available in the literature are discussed.
2016-01-09
studied in detail using scanning tunneling microscopy and angle resolved photoemission. For the doping levels achieved in cobalt titanium antimony, the...angle resolved photoemission. For the doping levels achieved in cobalt titanium antimony, the electron mobility at room temperature was comparable...scanning tunneling microscopy and angle resolved photoemission. For the doping levels achieved in cobalt titanium antimony, the electron mobility at room
NASA Astrophysics Data System (ADS)
Wu, Heng
2000-10-01
In this thesis, an a-posteriori error estimator is presented and employed for solving viscous incompressible flow problems. In an effort to detect local flow features, such as vortices and separation, and to resolve flow details precisely, a velocity angle error estimator e theta which is based on the spatial derivative of velocity direction fields is designed and constructed. The a-posteriori error estimator corresponds to the antisymmetric part of the deformation-rate-tensor, and it is sensitive to the second derivative of the velocity angle field. Rationality discussions reveal that the velocity angle error estimator is a curvature error estimator, and its value reflects the accuracy of streamline curves. It is also found that the velocity angle error estimator contains the nonlinear convective term of the Navier-Stokes equations, and it identifies and computes the direction difference when the convective acceleration direction and the flow velocity direction have a disparity. Through benchmarking computed variables with the analytic solution of Kovasznay flow or the finest grid of cavity flow, it is demonstrated that the velocity angle error estimator has a better performance than the strain error estimator. The benchmarking work also shows that the computed profile obtained by using etheta can achieve the best matching outcome with the true theta field, and that it is asymptotic to the true theta variation field, with a promise of fewer unknowns. Unstructured grids are adapted by employing local cell division as well as unrefinement of transition cells. Using element class and node class can efficiently construct a hierarchical data structure which provides cell and node inter-reference at each adaptive level. Employing element pointers and node pointers can dynamically maintain the connection of adjacent elements and adjacent nodes, and thus avoids time-consuming search processes. The adaptive scheme is applied to viscous incompressible flow at different Reynolds numbers. It is found that the velocity angle error estimator can detect most flow characteristics and produce dense grids in the regions where flow velocity directions have abrupt changes. In addition, the e theta estimator makes the derivative error dilutely distribute in the whole computational domain and also allows the refinement to be conducted at regions of high error. Through comparison of the velocity angle error across the interface with neighbouring cells, it is verified that the adaptive scheme in using etheta provides an optimum mesh which can clearly resolve local flow features in a precise way. The adaptive results justify the applicability of the etheta estimator and prove that this error estimator is a valuable adaptive indicator for the automatic refinement of unstructured grids.
Nanomechanical effects of light unveil photons momentum in medium
Verma, Gopal; Chaudhary, Komal; Singh, Kamal P.
2017-01-01
Precision measurement on momentum transfer between light and fluid interface has many implications including resolving the intriguing nature of photons momentum in a medium. For example, the existence of Abraham pressure of light under specific experimental configuration and the predictions of Chau-Amperian formalism of optical momentum for TE and TM polarizations remain untested. Here, we quantitatively and cleanly measure nanomehanical dynamics of water surface excited by radiation pressure of a laser beam. We systematically scanned wide range of experimental parameters including long exposure times, angle of incidence, spot size and laser polarization, and used two independent pump-probe techniques to validate a nano- bump on the water surface under all the tested conditions, in quantitative agreement with the Minkowski’s momentum of light. With careful experiments, we demonstrate advantages and limitations of nanometer resolved optical probing techniques and narrow down actual manifestation of optical momentum in a medium. PMID:28198468
Highly Charged Rydberg Ions from the Coulomb Explosion of Clusters
NASA Astrophysics Data System (ADS)
Komar, D.; Kazak, L.; Almassarani, M.; Meiwes-Broer, K.-H.; Tiggesbäumker, J.
2018-03-01
Ion emission from a nanoplasma produced in the interaction of intense optical laser pulses with argon clusters is studied resolving simultaneously charge states and recoil energies. By applying appropriate static electric fields we observe that a significant fraction of the ions Arq + (q =1 - 7 ) has electrons with binding energies lower than 150 meV; i.e., nRyd≥15 levels are populated. Charge state changes observed on a μ s time scale can be attributed to electron emission due to autoionizing Rydberg states, indicating that high-ℓ Rydberg levels are populated as well. The experiments support theoretical predictions that a significant fraction of delocalized electrons, which are bound with hundreds of eV to the nanoplasma after the laser exposure, fill up meV bound ion states in the adiabatic expansion. We expect the process to be relevant for the long-term evolution of expanding laser-induced dense plasmas in general.
NASA Technical Reports Server (NTRS)
Pang, Yong; Lefskky, Michael; Sun, Guoqing; Ranson, Jon
2011-01-01
A spaceborne lidar mission could serve multiple scientific purposes including remote sensing of ecosystem structure, carbon storage, terrestrial topography and ice sheet monitoring. The measurement requirements of these different goals will require compromises in sensor design. Footprint diameters that would be larger than optimal for vegetation studies have been proposed. Some spaceborne lidar mission designs include the possibility that a lidar sensor would share a platform with another sensor, which might require off-nadir pointing at angles of up to 16 . To resolve multiple mission goals and sensor requirements, detailed knowledge of the sensitivity of sensor performance to these aspects of mission design is required. This research used a radiative transfer model to investigate the sensitivity of forest height estimates to footprint diameter, off-nadir pointing and their interaction over a range of forest canopy properties. An individual-based forest model was used to simulate stands of mixed conifer forest in the Tahoe National Forest (Northern California, USA) and stands of deciduous forests in the Bartlett Experimental Forest (New Hampshire, USA). Waveforms were simulated for stands generated by a forest succession model using footprint diameters of 20 m to 70 m. Off-nadir angles of 0 to 16 were considered for a 25 m diameter footprint diameter. Footprint diameters in the range of 25 m to 30 m were optimal for estimates of maximum forest height (R(sup 2) of 0.95 and RMSE of 3 m). As expected, the contribution of vegetation height to the vertical extent of the waveform decreased with larger footprints, while the contribution of terrain slope increased. Precision of estimates decreased with an increasing off-nadir pointing angle, but off-nadir pointing had less impact on height estimates in deciduous forests than in coniferous forests. When pointing off-nadir, the decrease in precision was dependent on local incidence angle (the angle between the off-nadir beam and a line normal to the terrain surface) which is dependent on the off-nadir pointing angle, terrain slope, and the difference between the laser pointing azimuth and terrain aspect; the effect was larger when the sensor was aligned with the terrain azimuth but when aspect and azimuth are opposed, there was virtually no effect on R2 or RMSE. A second effect of off-nadir pointing is that the laser beam will intersect individual crowns and the canopy as a whole from a different angle which had a distinct effect on the precision of lidar estimates of height, decreasing R2 and increasing RMSE, although the effect was most pronounced for coniferous crowns.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Holmgren, D.E.; Walker, D.J.; Harris, S.E.
Certain quartet levels in alkali-like systems retain metastability against autoionization while acquiring large radiative yields. This quasi-metastability occurs through selective coupling to non-autoionizing doublet levels by the spin-orbit interaction. An example of such a level is the 5p/sup 5/5d6s /sup 4/P/sub 5/2/ level of neutral Cs, which has a calculated branching ratio for radiation at 1091 A of 43%. Experimentally, we find that this line has an emission intensity equal to 1/6 of that of the strongest ion line of Cs/sup +/, and is a promising candidate for an extreme ultraviolet laser.
Charge-transfer dynamics in one-dimensional C 60 chains
NASA Astrophysics Data System (ADS)
Pérez-Dieste, V.; Tamai, A.; Greber, T.; Chiuzbaˇian, S. G.; Patthey, L.
2008-06-01
Charge transfer in highly-ordered C 60 chains grown on a Cu(5 5 3) vicinal surface is studied by means of resonant photoemission. Tuning the light polarization, autoionization of the highest occupied molecular orbital (HOMO) was expected to detect anisotropy in this one-dimensional system. For one monolayer C 60 we found no signature of autoionization. This indicates that for an electron which is excited from the C 1s level of C 60 to the lowest unoccupied molecular orbital (LUMO), hybridization leads to delocalization on the femtosecond time-scale and no influence of the light polarization is observed.
EFFECTS OF LASER RADIATION ON MATTER: Spectrum of the barium atom in a laser radiation field
NASA Astrophysics Data System (ADS)
Bondar', I. I.; Suran, V. V.
1990-08-01
An experimental investigation was made of the influence of a laser radiation field on the spectrum of barium atoms. The investigation was carried out by the method of three-photon ionization spectroscopy using dye laser radiation (ω = 14 800-18 700 cm - 1). The electric field intensity of the laser radiation was 103-106 V/cm. This laser radiation field had a strong influence on a number of bound and autoionizing states. The nature of this influence depended on the ratio of the excitation frequencies of bound and autoionizing states.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Sun, Xuan; Zhang, Wen-Tao; Zhao, Lin
For this study, we carry out detailed momentum-dependent and temperature-dependent measurements on Bi 2Sr 2CaCu 2O 8+δ (Bi2212) superconductor in the superconducting and pseudogap states by super-high resolution laser-based angle-resolved photoemission spectroscopy. The precise determination of the superconducting gap for the nearly optimally doped Bi2212 (T c=91 K) at low temperature indicates that the momentum-dependence of the superconducting gap deviates from the standard d-wave form (cos(2Φ)). It can be alternatively fitted by including a high-order term (cos(6Φ)) in which the next nearest-neighbor interaction is considered. We find that the band structure near the antinodal region smoothly evolves across the pseudogapmore » temperature without a signature of band reorganization which is distinct from that found in Bi 2Sr 2CuO 6+δ superconductors. This indicates that the band reorganization across the pseudogap temperature is not a universal behavior in cuprate superconductors. These results provide new insights in understanding the nature of the superconducting gap and pseudogap in high-temperature cuprate superconductors.« less
Sun, Xuan; Zhang, Wen-Tao; Zhao, Lin; ...
2017-12-17
For this study, we carry out detailed momentum-dependent and temperature-dependent measurements on Bi 2Sr 2CaCu 2O 8+δ (Bi2212) superconductor in the superconducting and pseudogap states by super-high resolution laser-based angle-resolved photoemission spectroscopy. The precise determination of the superconducting gap for the nearly optimally doped Bi2212 (T c=91 K) at low temperature indicates that the momentum-dependence of the superconducting gap deviates from the standard d-wave form (cos(2Φ)). It can be alternatively fitted by including a high-order term (cos(6Φ)) in which the next nearest-neighbor interaction is considered. We find that the band structure near the antinodal region smoothly evolves across the pseudogapmore » temperature without a signature of band reorganization which is distinct from that found in Bi 2Sr 2CuO 6+δ superconductors. This indicates that the band reorganization across the pseudogap temperature is not a universal behavior in cuprate superconductors. These results provide new insights in understanding the nature of the superconducting gap and pseudogap in high-temperature cuprate superconductors.« less
Gong, Xuepeng; Lu, Qipeng
2015-01-01
A new monochromator is designed to develop a high performance soft X-ray microscopy beamline at Shanghai Synchrotron Radiation Facility (SSRF). But owing to its high resolving power and high accurate spectrum output, there exist many technical difficulties. In the paper presented, as two primary design targets for the monochromator, theoretical energy resolution and photon flux of the beamline are calculated. For wavelength scanning mechanism, primary factors affecting the rotary angle errors are presented, and the measuring results are 0.15'' and 0.17'' for plane mirror and plane grating, which means that it is possible to provide sufficient scanning precision to specific wavelength. For plane grating switching mechanism, the repeatabilities of roll, yaw and pitch angles are 0.08'', 0.12'' and 0.05'', which can guarantee the high accurate switch of the plane grating effectively. After debugging, the repeatability of light spot drift reaches to 0.7'', which further improves the performance of the monochromator. The commissioning results show that the energy resolving power is higher than 10000 at Ar L-edge, the photon flux is higher than 1 × 108 photons/sec/200 mA, and the spatial resolution is better than 30 nm, demonstrating that the monochromator performs very well and reaches theoretical predictions.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Evans, M.; Ng, C.Y.
1999-11-01
We have obtained rotationally resolved pulsed field ionization{endash}photoelectron (PFI-PE) spectra of CO in the energy range of 13.98{endash}21.92 eV, covering the ionization transitions CO{sup +}(X&hthinsp;{sup 2}{Sigma}{sup +},v{sup +}=0{endash}42,N{sup +}){l_arrow}CO(X&hthinsp;{sup 1}{Sigma}{sup +},v{sup {double_prime}}=0,N{sup {double_prime}}). The PFI-PE bands for CO{sup +}&hthinsp;(X&hthinsp;{sup 2}{Sigma}{sup +}, v{sup +}=8{endash}22, 24, and 28{endash}39) obtained here represent the first rotationally resolved spectroscopic data for these states. The high-resolution features observed in the PFI-PE spectra allow the identification of vibrational bands for the CO{sup +}&hthinsp;(X&hthinsp;{sup 2}{Sigma}{sup +}, v{sup +}=10, 14, 15, 17, 18, 21, 24, 25, 29{endash}31, 33, 35{endash}37, and 39) states, which strongly overlap with prominent vibrational bandsmore » of the CO{sup +}(A&hthinsp;{sup 2}{Pi}{sub 3/2,1/2},B&hthinsp;{sup 2}{Sigma}{sup +}) states. The simulation using the Buckingham{endash}Orr{endash}Sichel model has provided accurate molecular constants for CO{sup +}(X&hthinsp;{sup 2}{Sigma}{sup +},v{sup +}=0{endash}42), including ionization energies, vibrational constants ({omega}{sub e}{sup +}=2218.8{plus_minus}3.5&hthinsp;cm{sup {minus}1}, {omega}{sub e}{sup +}x{sub e}{sup +}=16.20{plus_minus}0.32&hthinsp;cm{sup {minus}1}, {omega}{sub e}{sup +}y{sub e}{sup +}=0.074{plus_minus}0.011&hthinsp;cm{sup {minus}1}, and {omega}{sub e}{sup +}z{sub e}{sup +}={minus}0.001&hthinsp;83{plus_minus}0.000&hthinsp;13&hthin p;cm{sup {minus}1}), and rotational constants [B{sub e}{sup +}=1.9797{plus_minus}0.0051&hthinsp;cm{sup {minus}1}, {alpha}{sub e}{sup +}=0.0201{plus_minus}0.0011thinspcm{sup {minus}1}, {gamma}{sub e}{sup +}=0.000&hthinsp;122{plus_minus}0.000&hthinsp;067&hthinsp;cm{sup {minus}1}, z{sub e}{sup +}={minus}(5.2{plus_minus}1.1){times}10{sup {minus}6}&hthinsp;cm{sup {minus}1}]. Enhancement of {Delta}N{lt}0 rotational branches, attributable to field-induced rotational autoionization, was clearly discernible in PFI-PE bands for CO{sup +}&hthinsp;(X&hthinsp;{sup 2}{Sigma}{sup +}, v{sup +}=0{endash}5, 11, and 12). Significant local enhancements due to near-resonance autoionization were observed for low v{sup +} ({lt}10) PFI-PE bands of CO{sup +}(X&hthinsp;{sup 2}{Sigma}{sup +}), where the density of interloper Rydberg states converging to higher ionic levels is high as manifested in the photoion spectrum. The observation of a long vibrational progression in the Franck{endash}Condon gap region, where strong autoionization states are absent, is consistent with the suggestion that high-{ital n} Rydberg states converging to highly excited vibrational levels of CO{sup +}(X&hthinsp;{sup 2}{Sigma}{sup +}) are partially populated via direct excitation to a repulsive neutral state. The relatively minor band intensity variation observed for high v{sup +} PFI-PE bands is also in accord with the direct excitation model. Since {Delta}N=0, {plus_minus}1, {plus_minus}2, and {plus_minus}3 rotational branches are observed in the PFI-PE spectra, we conclude that the ejected photoelectrons are restricted to angular momentum continuum states l=0{endash}4. {copyright} {ital 1999 American Institute of Physics.}« less
Design of a self-calibration high precision micro-angle deformation optical monitoring scheme
NASA Astrophysics Data System (ADS)
Gu, Yingying; Wang, Li; Guo, Shaogang; Wu, Yun; Liu, Da
2018-03-01
In order to meet the requirement of high precision and micro-angle measurement on orbit, a self-calibrated optical non-contact real-time monitoring device is designed. Within three meters, the micro-angle variable of target relative to measuring basis can be measured in real-time. The range of angle measurement is +/-50'', the angle measurement accuracy is less than 2''. The equipment can realize high precision real-time monitoring the micro-angle deformation, which caused by high strength vibration and shock of rock launching, sun radiation and heat conduction on orbit and so on.
How to measure separations and angles between intra-molecular fluorescent markers
NASA Astrophysics Data System (ADS)
Flyvbjerg, Henrik; Mortensen, Kim I.; Sung, Jongmin; Spudich, James A.
We demonstrate a novel, yet simple tool for the study of structure and function of biomolecules by extending two-colour co-localization microscopy to fluorescent molecules with fixed orientations and in intra-molecular proximity. From each color-separated microscope image in a time-lapse movie and using only simple means, we simultaneously determine both the relative (x,y)-separation of the fluorophores and their individual orientations in space with accuracy and precision. The positions and orientations of two domains of the same molecule are thus time-resolved. Using short double-stranded DNA molecules internally labelled with two fixed fluorophores, we demonstrate the accuracy and precision of our method using the known structure of double-stranded DNA as a benchmark, resolve 10-base-pair differences in fluorophore separations, and determine the unique 3D orientation of each DNA molecule, thereby establishing short, double-labelled DNA molecules as probes of 3D orientation of anything to which one can attach them firmly. This work was supported by a Lundbeck fellowship to K.I.M; a Stanford Bio-X fellowship to J.S. and Grants from the NIH (GM33289) to J.A.S. and the Human Frontier Science Program (GP0054/2009-C) to J.A.S. and H.F.
Second Class Resolver: a retrospective analysis.
D'Attilio, M; Rodolfino, D; Filippakos, A; Saccucci, M; Festa, F; Tripodi, D
2014-03-01
To evaluate the use of Second Class Resolver (SCR), a new fixed orthopaedic appliance, for the treatment of skeletal Class II malocclusion in growing subjects. Design Retrospective analysis. Forty subjects were treated with Second Class Resolver (SCR). The mean age was 8 years at the beginning of treatment and 10 years at the end of treatment. Digital cephalometric superimpositions on lateral radiographs taken at start and end of treatment were assessed. The cephalometric values were statistically analysed. Cephalometric analysis of changes during treatment shows reduction of ANB angle (mean 2°); reduction of Witts Index (mean 3 mm); reduction of Maxillo-Mandibular angle (MM) (mean 1°); reduction of SNA (angle mean 3°); reduction of gonial angle (mean 1.8°); increase of the mandibular branch length (mean 5 mm); increase of mandibular body (mean 2.9°). The Second Class Resolver can be beneficially used for the treatment of Class II malocclusion.
Wigner-Eisenbud-Smith photoionization time delay due to autoioinization resonances
NASA Astrophysics Data System (ADS)
Deshmukh, P. C.; Kumar, A.; Varma, H. R.; Banerjee, S.; Manson, Steven T.; Dolmatov, V. K.; Kheifets, A. S.
2018-03-01
An empirical ansatz for the complex photoionization amplitude and Wigner-Eisenbud-Smith time delay in the vicinity of a Fano autoionization resonance are proposed to evaluate and interpret the time delay in the resonant region. The utility of this expression is evaluated in comparison with accurate numerical calculations employing the ab initio relativistic random phase approximation and relativistic multichannel quantum defect theory. The indisputably good qualitative agreement (and semiquantitative agreement) between corresponding results of the proposed model and results produced by the ab initio theories proves the usability of the model. In addition, the phenomenology of the time delay in the vicinity of multichannel autoionizing resonances is detailed.
NASA Astrophysics Data System (ADS)
Chu, Wei-Chun; Lin, C. D.
2013-01-01
An extreme ultraviolet (EUV) single attosecond pulse passing through a laser-dressed dense gas is studied theoretically. The weak EUV pulse pumps the helium gas from the ground state to the 2s2p(1P) autoionizing state, which is coupled to the 2s2(1S) autoionizing state by a femtosecond infrared laser with the intensity in the order of 1012 W/cm2. The simulation shows how the transient absorption and emission of the EUV are modified by the coupling laser. A simple analytical expression for the atomic response derived for δ-function pulses reveals the strong modification of the Fano lineshape in the spectra, where these features are quite universal and remain valid for realistic pulse conditions. We further account for the propagation of pulses in the medium and show that the EUV signal at the atomic resonance can be enhanced in the gaseous medium by more than 50% for specifically adjusted laser parameters, and that this enhancement persists as the EUV propagates in the gaseous medium. Our result demonstrates the high-level control of nonlinear optical effects that are achievable with attosecond pulses.
NASA Astrophysics Data System (ADS)
Glushkov, Alexander; Loboda, Andrey; Nikola, Ludmila
2011-10-01
We present the uniform energy approach, formally based on the gauge-invariant relativistic many-body perturbation theory for the calculation of the radiative and autoionization probabilities, electron collision strengths and rate coefficients in a multicharged ions (in a collisionally pumped plasma). An account for the plasma medium influence is carried out within a Debae shielding approach. The aim is to study, in a uniform manner, elementary processes responsible for emission-line formation in a plasma. The energy shift due to the collision is arisen at first in the second PT order in the form of integral on the scattered electron energy. The cross-section is linked with imaginary part of the scattering energy shift. The electron collision excitation cross-sections and rate coefficients for some plasma Ne-, Ar-like multicharged ions are calculated within relativistic energy approach. We present the results of calculation the autoionization resonances energies and widths in heavy He-like multicharged ions and rare-earth atoms of Gd and Tm. To test the results of calculations we compare the obtained data for some Ne-like ions with other authors' calculations and available experimental data for a wide range of plasma conditions.
High-order harmonic generation from highly excited states in acetylene
NASA Astrophysics Data System (ADS)
Mulholland, Peter; Dundas, Daniel
2018-04-01
High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are described using time-dependent density-functional theory while the ions are treated classically. We find that for molecules aligned perpendicular to the laser polarization axis, HHG arises from the highest-occupied molecular orbital (HOMO), while for molecules aligned along the laser polarization axis, HHG is dominated by the HOMO-1. In the parallel orientation we observe a double plateau with an inner plateau that is produced by ionization from and recombination back to an autoionizing state. Two pieces of evidence support this idea. First, by choosing a suitably tuned vacuum ultraviolet pump pulse that directly excites the autoionizing state we observe a dramatic enhancement of all harmonics in the inner plateau. Second, in certain circumstances, the position of the inner plateau cutoff does not agree with the classical three-step model. We show that this discrepancy can be understood in terms of a minimum in the dipole recombination matrix element from the continuum to the autoionizing state.
UV + V UV double-resonance studies of autoionizing Rydberg states of the hydroxyl radical
DOE Office of Scientific and Technical Information (OSTI.GOV)
Green, Amy M.; Liu, Fang; Lester, Marsha I., E-mail: milester@sas.upenn.edu
2016-05-14
The hydroxyl radical (OH) is a key oxidant in atmospheric and combustion chemistry. Recently, a sensitive and state-selective ionization method has been developed for detection of the OH radical that utilizes UV excitation on the A{sup 2}Σ{sup +}–X{sup 2}Π transition followed by fixed 118 nm vacuum ultraviolet (VUV) radiation to access autoionizing Rydberg states [J. M. Beames et al., J. Chem. Phys. 134, 241102 (2011)]. The present study uses tunable VUV radiation generated by four-wave mixing to examine the origin of the enhanced ionization efficiency observed for OH radicals prepared in specific A{sup 2}Σ{sup +} intermediate levels. The enhancement ismore » shown to arise from resonant excitation to distinct rotational and fine structure levels of two newly identified {sup 2}Π Rydberg states with an A{sup 3}Π cationic core and a 3d electron followed by ionization. Spectroscopic constants are derived and effects due to uncoupling of the Rydberg electron are revealed for the OH {sup 2}Π Rydberg states. The linewidths indicate a Rydberg state lifetime due to autoionization on the order of a picosecond.« less
Angle-resolved diffraction grating biosensor based on porous silicon
DOE Office of Scientific and Technical Information (OSTI.GOV)
Lv, Changwu; Li, Peng; Jia, Zhenhong, E-mail: jzhh@xju.edu.cn
2016-03-07
In this study, an optical biosensor based on a porous silicon composite structure was fabricated using a simple method. This structure consists of a thin, porous silicon surface diffraction grating and a one-dimensional porous silicon photonic crystal. An angle-resolved diffraction efficiency spectrum was obtained by measuring the diffraction efficiency at a range of incident angles. The angle-resolved diffraction efficiency of the 2nd and 3rd orders was studied experimentally and theoretically. The device was sensitive to the change of refractive index in the presence of a biomolecule indicated by the shift of the diffraction efficiency spectrum. The sensitivity of this sensormore » was investigated through use of an 8 base pair antifreeze protein DNA hybridization. The shifts of the angle-resolved diffraction efficiency spectrum showed a relationship with the change of the refractive index, and the detection limit of the biosensor reached 41.7 nM. This optical device is highly sensitive, inexpensive, and simple to fabricate. Using shifts in diffraction efficiency spectrum to detect biological molecules has not yet been explored, so this study establishes a foundation for future work.« less
Difference structures from time-resolved small-angle and wide-angle x-ray scattering
NASA Astrophysics Data System (ADS)
Nepal, Prakash; Saldin, D. K.
2018-05-01
Time-resolved small-angle x-ray scattering/wide-angle x-ray scattering (SAXS/WAXS) is capable of recovering difference structures directly from difference SAXS/WAXS curves. It does so by means of the theory described here because the structural changes in pump-probe detection in a typical time-resolved experiment are generally small enough to be confined to a single residue or group in close proximity which is identified by a method akin to the difference Fourier method of time-resolved crystallography. If it is assumed, as is usual with time-resolved structures, that the moved atoms lie within the residue, the 100-fold reduction in the search space (assuming a typical protein has about 100 residues) allows the exaction of the structure by a simulated annealing algorithm with a huge reduction in computing time and leads to a greater resolution by varying the positions of atoms only within that residue. This reduction in the number of potential moved atoms allows us to identify the actual motions of the individual atoms. In the case of a crystal, time-resolved calculations are normally performed using the difference Fourier method, which is, of course, not directly applicable to SAXS/WAXS. The method developed in this paper may be thought of as a substitute for that method which allows SAXS/WAXS (and hence disordered molecules) to also be used for time-resolved structural work.
Apparatus and method for variable angle slant hole collimator
Lee, Seung Joon; Kross, Brian J.; McKisson, John E.
2017-07-18
A variable angle slant hole (VASH) collimator for providing collimation of high energy photons such as gamma rays during radiological imaging of humans. The VASH collimator includes a stack of multiple collimator leaves and a means of quickly aligning each leaf to provide various projection angles. Rather than rotate the detector around the subject, the VASH collimator enables the detector to remain stationary while the projection angle of the collimator is varied for tomographic acquisition. High collimator efficiency is achieved by maintaining the leaves in accurate alignment through the various projection angles. Individual leaves include unique angled cuts to maintain a precise target collimation angle. Matching wedge blocks driven by two actuators with twin-lead screws accurately position each leaf in the stack resulting in the precise target collimation angle. A computer interface with the actuators enables precise control of the projection angle of the collimator.
Fat fraction bias correction using T1 estimates and flip angle mapping.
Yang, Issac Y; Cui, Yifan; Wiens, Curtis N; Wade, Trevor P; Friesen-Waldner, Lanette J; McKenzie, Charles A
2014-01-01
To develop a new method of reducing T1 bias in proton density fat fraction (PDFF) measured with iterative decomposition of water and fat with echo asymmetry and least-squares estimation (IDEAL). PDFF maps reconstructed from high flip angle IDEAL measurements were simulated and acquired from phantoms and volunteer L4 vertebrae. T1 bias was corrected using a priori T1 values for water and fat, both with and without flip angle correction. Signal-to-noise ratio (SNR) maps were used to measure precision of the reconstructed PDFF maps. PDFF measurements acquired using small flip angles were then compared to both sets of corrected large flip angle measurements for accuracy and precision. Simulations show similar results in PDFF error between small flip angle measurements and corrected large flip angle measurements as long as T1 estimates were within one standard deviation from the true value. Compared to low flip angle measurements, phantom and in vivo measurements demonstrate better precision and accuracy in PDFF measurements if images were acquired at a high flip angle, with T1 bias corrected using T1 estimates and flip angle mapping. T1 bias correction of large flip angle acquisitions using estimated T1 values with flip angle mapping yields fat fraction measurements of similar accuracy and superior precision compared to low flip angle acquisitions. Copyright © 2013 Wiley Periodicals, Inc.
Fang, Ning; Sun, Wei
2015-04-21
A method, apparatus, and system for improved VA-TIRFM microscopy. The method comprises automatically controlled calibration of one or more laser sources by precise control of presentation of each laser relative a sample for small incremental changes of incident angle over a range of critical TIR angles. The calibration then allows precise scanning of the sample for any of those calibrated angles for higher and more accurate resolution, and better reconstruction of the scans for super resolution reconstruction of the sample. Optionally the system can be controlled for incident angles of the excitation laser at sub-critical angles for pseudo TIRFM. Optionally both above-critical angle and sub critical angle measurements can be accomplished with the same system.
NASA Astrophysics Data System (ADS)
Kraus, D.; Hartley, N. J.; Frydrych, S.; Schuster, A. K.; Rohatsch, K.; Rödel, M.; Cowan, T. E.; Brown, S.; Cunningham, E.; van Driel, T.; Fletcher, L. B.; Galtier, E.; Gamboa, E. J.; Laso Garcia, A.; Gericke, D. O.; Granados, E.; Heimann, P. A.; Lee, H. J.; MacDonald, M. J.; MacKinnon, A. J.; McBride, E. E.; Nam, I.; Neumayer, P.; Pak, A.; Pelka, A.; Prencipe, I.; Ravasio, A.; Redmer, R.; Saunders, A. M.; Schölmerich, M.; Schörner, M.; Sun, P.; Turner, S. J.; Zettl, A.; Falcone, R. W.; Glenzer, S. H.; Döppner, T.; Vorberger, J.
2018-05-01
Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.
Non-LTE profiles of the Al I autoionization lines. [for solar model atmospheres
NASA Technical Reports Server (NTRS)
Finn, G. D.; Jefferies, J. T.
1974-01-01
A non-LTE formulation is given for the transfer of radiation in the autoionizing lines of neutral aluminum at 1932 and 1936 A through both the Bilderberg and Harvard-Smithsonian model atmospheres. Numerical solutions for the common source function of these lines and their theoretical line profiles are calculated and compared with the corresponding LTE profiles. The results show that the non-LTE profiles provide a better match with the observations. They also indicate that the continuous opacity of the standard solar models should be increased in this wavelength region if the center-limb variations of observed and theoretical profiles of these lines are to be in reasonable agreement.
NASA Astrophysics Data System (ADS)
Högström, Jonas; Fredriksson, Wendy; Edstrom, Kristina; Björefors, Fredrik; Nyholm, Leif; Olsson, Claes-Olof A.
2013-11-01
An approach for determining depth gradients of metal-ion concentrations in passive films on stainless steel using angle-resolved X-ray photoelectron spectroscopy (ARXPS) is described. The iterative method, which is based on analyses of the oxidised metal peaks, provides increased precision and hence allows faster ARXPS measurements to be carried out. The method was used to determine the concentration depth profiles for molybdenum, iron and chromium in passive films on 316L/EN 1.4432 stainless steel samples oxidised in 0.5 M H2SO4 and acetic acid diluted with 0.02 M Na2B4O7 · 10H2O and 1 M H2O, respectively. The molybdenum concentration in the film is pin-pointed to the oxide/metal interface and the films also contained an iron-ion-enriched surface layer and a chromium-ion-dominated middle layer. Although films of similar composition and thickness (i.e., about 2 nm) were formed in the two electrolytes, the corrosion currents were found to be three orders of magnitude larger in the acetic acid solution. The differences in the layer composition, found for the two electrolytes as well as different oxidation conditions, can be explained based on the oxidation potentials of the metals and the dissolution rates of the different metal ions.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Sato, Soshi, E-mail: sato.soshi@cies.tohoku.ac.jp; Honjo, Hiroaki; Niwa, Masaaki
2015-04-06
We have investigated the redox reaction on the surface of Ta/CoFeB/MgO/CoFeB magnetic tunnel junction stack samples after annealing at 300, 350, and 400 °C for 1 h using angle-resolved X-ray photoelectron spectroscopy for precise analysis of the chemical bonding states. At a capping tantalum layer thickness of 1 nm, both the capping tantalum layer and the surface of the underneath CoFeB layer in the as-deposited stack sample were naturally oxidized. By comparison of the Co 2p and Fe 2p spectra among the as-deposited and annealed samples, reduction of the naturally oxidized cobalt and iron atoms occurred on the surface of the CoFeB layer.more » The reduction reaction was more significant at higher annealing temperature. Oxidized cobalt and iron were reduced by boron atoms that diffused toward the surface of the top CoFeB layer. A single CoFeB layer was prepared on SiO{sub 2}, and a confirmatory evidence of the redox reaction with boron diffusion was obtained by angle-resolved X-ray photoelectron spectroscopy analysis of the naturally oxidized surface of the CoFeB single layer after annealing. The redox reaction is theoretically reasonable based on the Ellingham diagram.« less
Anisotropic interactions of a single spin and dark-spin spectroscopy in diamond
NASA Astrophysics Data System (ADS)
Epstein, R. J.; Mendoza, F. M.; Kato, Y. K.; Awschalom, D. D.
2005-11-01
Experiments on single nitrogen-vacancy (N-V) centres in diamond, which include electron spin resonance, Rabi oscillations, single-shot spin readout and two-qubit operations with a nearby13C nuclear spin, show the potential of this spin system for solid-state quantum information processing. Moreover, N-V centre ensembles can have spin-coherence times exceeding 50 μs at room temperature. We have developed an angle-resolved magneto-photoluminescence microscope apparatus to investigate the anisotropic electron-spin interactions of single N-V centres at room temperature. We observe negative peaks in the photoluminescence as a function of both magnetic-field magnitude and angle that are explained by coherent spin precession and anisotropic relaxation at spin-level anti-crossings. In addition, precise field alignment unmasks the resonant coupling to neighbouring `dark' nitrogen spins, otherwise undetected by photoluminescence. These results demonstrate the capability of our spectroscopic technique for measuring small numbers of dark spins by means of a single bright spin under ambient conditions.
Investigations of interpolation errors of angle encoders for high precision angle metrology
NASA Astrophysics Data System (ADS)
Yandayan, Tanfer; Geckeler, Ralf D.; Just, Andreas; Krause, Michael; Asli Akgoz, S.; Aksulu, Murat; Grubert, Bernd; Watanabe, Tsukasa
2018-06-01
Interpolation errors at small angular scales are caused by the subdivision of the angular interval between adjacent grating lines into smaller intervals when radial gratings are used in angle encoders. They are often a major error source in precision angle metrology and better approaches for determining them at low levels of uncertainty are needed. Extensive investigations of interpolation errors of different angle encoders with various interpolators and interpolation schemes were carried out by adapting the shearing method to the calibration of autocollimators with angle encoders. The results of the laboratories with advanced angle metrology capabilities are presented which were acquired by the use of four different high precision angle encoders/interpolators/rotary tables. State of the art uncertainties down to 1 milliarcsec (5 nrad) were achieved for the determination of the interpolation errors using the shearing method which provides simultaneous access to the angle deviations of the autocollimator and of the angle encoder. Compared to the calibration and measurement capabilities (CMC) of the participants for autocollimators, the use of the shearing technique represents a substantial improvement in the uncertainty by a factor of up to 5 in addition to the precise determination of interpolation errors or their residuals (when compensated). A discussion of the results is carried out in conjunction with the equipment used.
Efficient mass-selective three-photon ionization of zirconium atoms
Page, Ralph H.
1994-01-01
In an AVLIS process, .sup.91 Zr is selectively removed from natural zirconium by a three-step photoionization wherein Zr atoms are irradiated by a laser beam having a wavelength .lambda..sub.1, selectively raising .sup.91 Zr atoms to an odd-parity E.sub.1 energy level in the range of 16000-19000 cm.sup.-1, are irradiated by a laser beam having a wavelength .lambda..sub.2 to raise the atoms from an E.sub.l level to an even-parity E.sub.2 energy level in the range of 35000-37000 cm.sup.-1 and are irradiated by a laser beam having a wavelength .lambda..sub.3 to cause a resonant transition of atoms from an E.sub.2 level to an autoionizing level above 53506 cm.sup.-1. .lambda..sub.3 wavelengths of 5607, 6511 or 5756 .ANG. will excite a zirconium atom from an E.sub.2 energy state of 36344 cm.sup.-1 to an autoionizing level; a .lambda..sub.3 wavelength of 5666 .ANG. will cause an autoionizing transition from an E.sub.2 level of 36068 cm.sup.-1 ; and a .lambda. .sub.3 wavelength of 5662 .ANG. will cause an ionizing resonance of an atom at an E.sub.2 level of 35904 cm.sup.-1.
Lubk, A; Rossell, M D; Seidel, J; He, Q; Yang, S Y; Chu, Y H; Ramesh, R; Hÿtch, M J; Snoeck, E
2012-07-27
Domain walls (DWs) substantially influence a large number of applications involving ferroelectric materials due to their limited mobility when shifted during polarization switching. The discovery of greatly enhanced conduction at BiFeO(3) DWs has highlighted yet another role of DWs as a local material state with unique properties. However, the lack of precise information on the local atomic structure is still hampering microscopical understanding of DW properties. Here, we examine the atomic structure of BiFeO(3) 109° DWs with pm precision by a combination of high-angle annular dark-field scanning transmission electron microscopy and a dedicated structural analysis. By measuring simultaneously local polarization and strain, we provide direct experimental proof for the straight DW structure predicted by ab initio calculations as well as the recently proposed theory of diffuse DWs, thus resolving a long-standing discrepancy between experimentally measured and theoretically predicted DW mobilities.
The star 12 Persei and separated fringe packet binaries (SFPB)
NASA Astrophysics Data System (ADS)
Bagnuolo, William G., Jr.; ten Brummelaar, Theo A.; McAlister, H. A.; Gies, Douglas R.; Ridgway, Stephen T.
2006-06-01
We have obtained high resolution orbital data with the CHARA Array for the bright star 12 Persei, a resolved double-lined spectroscopic binary, an example of a Separated Fringe Packet Binary. We describe the data reduction process involved. By using a technique we have developed of 'side-lobe verniering', we can obtain an improved precision in separation of up to 25 micro-arcsec along a given baseline. For this object we find a semi-major axis 0.3 of Barlow, Scarfe, and Fekel (1998) [BSF], but with an increased inclination angle. The revised masses are therefore almost 6% greater than those of BSF. The overall accuracy in the masses is about 1.3%, now primarily limited by the spectroscopically determined radial velocities. The precision of the masses due to the interferometrically derived "visual" orbit alone is only about 0.2%. We expect that improved RVs and improved absolute calibration can bring down the mass errors to below 1%.
[Evaluation of the resolving power of different angles in MPR images of 16DAS-MDCT].
Kimura, Mikio; Usui, Junshi; Nozawa, Takeo
2007-03-20
In this study, we evaluated the resolving power of three-dimensional (3D) multiplanar reformation (MPR) images with various angles by using 16 data acquisition system multi detector row computed tomography (16DAS-MDCT) . We reconstructed the MPR images using data with a 0.75 mm slice thickness of the axial image in this examination. To evaluate resolving power, we used an original new phantom (RC phantom) that can be positioned at any slice angle in MPR images. We measured the modulation transfer function (MTF) by using the methods of measuring pre-sampling MTF, and used Fourier transform of image data of the square wave chart. The scan condition and image reconstruction condition that were adopted in this study correspond to the condition that we use for three-dimensional computed tomographic angiography (3D-CTA) examination of the head in our hospital. The MTF of MPR images showed minimum values at slice angles in parallel with the axial slice, and showed maximum values at the sagittal slice and coronal slice angles that are parallel to the Z-axis. With an oblique MPR image, MTF did not change with angle changes in the oblique sagittal slice plane, but in the oblique coronal slice plane, MTF increased as the tilt angle increased from the axial plane to the Z plane. As a result, we could evaluate the resolving power of a head 3D image by measuring the MTF of the axial image and sagittal image or the coronal image.
Developing a clinically viable angle-resolved low coherence interferometry optical biopsy system
NASA Astrophysics Data System (ADS)
Pyhtila, John W.
2007-12-01
Non-invasive optical biopsy techniques, which interrogate tissue in situ, offer a potential method to improve the detection of dysplasia, a pre-cancerous tissue state. Specifically, monitoring of Barrett's esophagus (BE) patients for dysplasia, currently done through systematic biopsy, can be improved by increasing the proportion of at-risk tissue examined. Angle-resolved low coherence interferometry (a/LCI) is an optical spectroscopic technique which measures the depth resolved nuclear morphology of tissue, a key biomarker for identifying dysplasia. Using an animal carcinogenesis model, it was shown that a/LCI can detect dysplasia with great sensitivity and specificity. However, for the clinical application of a/LCI, numerous hurdles must be overcome. This dissertation presents the development of three new a/LCI systems which incrementally address the three main obstacles preventing the clinical application of a/LCI. First, data acquisition time is reduced by implementing a frequency-domain detection scheme using an imaging spectrograph that collects the complete depth resolved angular scattering distribution in parallel. This advance reduces data collection time to a clinically acceptable 40 ms. Second, a fiber probe is developed to enable the endoscopic application of a/LCI. The probe incorporates a single fiber for delivering light and a coherent fiber bundle for collecting the angular distribution of scattered light. Third, a portable device is created through miniaturization of the optical design, and a flexible fiber probe is created using polarization maintaining fiber to deliver the light. These advances allow for the clinical application of the system to ex vivo human tissue samples. The performance of each described system is evaluated through a number of validation studies, including the sizing of polystyrene microspheres, a typical model used in light scattering studies, and the measurement of in vitro cell nuclear diameters, accomplished with sub-wavelength precision and accuracy. The culmination of this work is the first human study using a/LCI in which it is demonstrated that a/LCI depth resolved nuclear morphology measurements provide an excellent means to identify dysplasia in BE patients. The described results demonstrate the great potential for the in vivo application of a/LCI as a targeting mechanism for the detection of dysplasia in Barrett's esophagus patients.
PRECISE ANGLE MONITOR BASED ON THE CONCEPT OF PENCIL-BEAM INTERFEROMETRY
DOE Office of Scientific and Technical Information (OSTI.GOV)
QIAN,S.; TAKACS,P.
2000-07-30
The precise angle monitoring is a very important metrology task for research, development and industrial applications. Autocollimator is one of the most powerful and widely applied instruments for small angle monitoring, which is based on the principle of geometric optics. In this paper the authors introduce a new precise angle monitoring system, Pencil-beam Angle Monitor (PAM), base on pencil beam interferometry. Its principle of operation is a combination of physical and geometrical optics. The angle calculation method is similar to the autocollimator. However, the autocollimator creates a cross image but the precise pencil-beam angle monitoring system produces an interference fringemore » on the focal plane. The advantages of the PAM are: high angular sensitivity, long-term stability character making angle monitoring over long time periods possible, high measurement accuracy in the order of sub-microradian, simultaneous measurement ability in two perpendicular directions or on two different objects, dynamic measurement possibility, insensitive to the vibration and air turbulence, automatic display, storage and analysis by use of the computer, small beam diameter making the alignment extremely easy and longer test distance. Some test examples are presented.« less
The Uncertainty of Local Background Magnetic Field Orientation in Anisotropic Plasma Turbulence
DOE Office of Scientific and Technical Information (OSTI.GOV)
Gerick, F.; Saur, J.; Papen, M. von, E-mail: felix.gerick@uni-koeln.de
In order to resolve and characterize anisotropy in turbulent plasma flows, a proper estimation of the background magnetic field is crucially important. Various approaches to calculating the background magnetic field, ranging from local to globally averaged fields, are commonly used in the analysis of turbulent data. We investigate how the uncertainty in the orientation of a scale-dependent background magnetic field influences the ability to resolve anisotropy. Therefore, we introduce a quantitative measure, the angle uncertainty, that characterizes the uncertainty of the orientation of the background magnetic field that turbulent structures are exposed to. The angle uncertainty can be used asmore » a condition to estimate the ability to resolve anisotropy with certain accuracy. We apply our description to resolve the spectral anisotropy in fast solar wind data. We show that, if the angle uncertainty grows too large, the power of the turbulent fluctuations is attributed to false local magnetic field angles, which may lead to an incorrect estimation of the spectral indices. In our results, an apparent robustness of the spectral anisotropy to false local magnetic field angles is observed, which can be explained by a stronger increase of power for lower frequencies when the scale of the local magnetic field is increased. The frequency-dependent angle uncertainty is a measure that can be applied to any turbulent system.« less
NASA Astrophysics Data System (ADS)
Jiang, Shanchao; Wang, Jing; Sui, Qingmei
2018-03-01
In order to achieve rotation angle measurement, one novel type of miniaturization fiber Bragg grating (FBG) rotation angle sensor with high measurement precision and temperature self-compensation is proposed and studied in this paper. The FBG rotation angle sensor mainly contains two core sensitivity elements (FBG1 and FBG2), triangular cantilever beam, and rotation angle transfer element. In theory, the proposed sensor can achieve temperature self-compensation by complementation of the two core sensitivity elements (FBG1 and FBG2), and it has a boundless angel measurement range with 2π rad period duo to the function of the rotation angle transfer element. Based on introducing the joint working processes, the theory calculation model of the FBG rotation angel sensor is established, and the calibration experiment on one prototype is also carried out to obtain its measurement performance. After experimental data analyses, the measurement precision of the FBG rotation angle sensor prototype is 0.2 ° with excellent linearity, and the temperature sensitivities of FBG1 and FBG2 are 10 pm/° and 10.1 pm/°, correspondingly. All these experimental results confirm that the FBG rotation angle sensor can achieve large-range angle measurement with high precision and temperature self-compensation.
Good, Philipp; Cooper, Thomas; Querci, Marco; Wiik, Nicolay; Ambrosetti, Gianluca; Steinfeld, Aldo
2016-03-01
The spectral specular reflectance of conventional and novel reflective materials for solar concentrators is measured with an acceptance angle of 17.5 mrad over the wavelength range 300-2500 nm at incidence angles 15-60° using a spectroscopic goniometry system. The same experimental setup is used to determine the spectral narrow-angle transmittance of semi-transparent materials for solar collector covers at incidence angles 0-60°. In addition, the angle-resolved surface scattering of reflective materials is recorded by an area-scan CCD detector over the spectral range 350-1050 nm. A comprehensive summary, discussion, and interpretation of the results are included in the associated research article "Spectral reflectance, transmittance, and angular scattering of materials for solar concentrators" in Solar Energy Materials and Solar Cells.
Angle-resolved PED and AED calculations for different structures of the diamond C(111) surface
NASA Astrophysics Data System (ADS)
Niebergall, L.; Rennert, P.; Chassé, A.; Kucherenko, Yu
1998-05-01
Angle-resolved (AR) photoelectron diffraction (PED) spectra for electrons excited from the C 1s core state and angle-resolved KVV Auger electron diffraction (AED) spectra are calculated for the Pandey and the Tsai stucture models of diamond C(111) which extend previous investigations of the ideal structure. It is shown how to decide on the structure model by comparing PE spectra for different directions and by comparing PED and AED spectra. Calculations have been performed by evaluating the scattering path operator for a finite cluster in a curved-wave approximation. The different matrix elements for the photoelectron excitation and for the Auger process, respectively, are included. It is shown that the PED intensities are very sensitive to the surface reconstruction for polar angles in the range of 80°. In the AED intensities, polar scans in the plane perpendicular to the chain direction can be considered.
The Origin of High-angle Dip-slip Earthquakes at Geothermal Fields in California
NASA Astrophysics Data System (ADS)
Barbour, A. J.; Schoenball, M.; Martínez-Garzón, P.; Kwiatek, G.
2016-12-01
We examine the source mechanisms of earthquakes occurring in three California geothermal fields: The Geysers, Salton Sea, and Coso. We find source mechanisms ranging from strike slip faulting, consistent with the tectonic settings, to dip slip with unusually steep dip angles which are inconsistent with local structures. For example, we identify a fault zone in the Salton Sea Geothermal Field imaged using precisely-relocated hypocenters with a dip angle of 60° yet double-couple focal mechanisms indicate higher-angle dip-slip on ≥75° dipping planes. We observe considerable temporal variability in the distribution of source mechanisms. For example, at the Salton Sea we find that the number of high angle dip-slip events increased after 1989, when net-extraction rates were highest. There is a concurrent decline in strike-slip and strike-slip-normal faulting, the mechanisms expected from regional tectonics. These unusual focal mechanisms and their spatio-temporal patterns are enigmatic in terms of our understanding of faulting in geothermal regions. While near-vertical fault planes are expected to slip in a strike-slip sense, and dip slip is expected to occur on moderately dipping faults, we observe dip slip on near-vertical fault planes. However, for plausible stress states and accounting for geothermal production, the resolved fault planes should be stable. We systematically analyze the source mechanisms of these earthquakes using full moment tensor inversion to understand the constraints imposed by assuming a double-couple source. Applied to The Geysers field, we find a significant reduction in the number of high-angle dip-slip mechanisms using the full moment tensor. The remaining mechanisms displaying high-angle dip-slip could be consistent with faults accommodating subsidence and compaction associated with volumetric strain changes in the geothermal reservoir.
Efficient mass-selective three-photon ionization of zirconium atoms
Page, R.H.
1994-12-27
In an AVLIS process, [sup 91]Zr is selectively removed from natural zirconium by a three-step photoionization wherein Zr atoms are irradiated by a laser beam having a wavelength [lambda][sub 1], selectively raising [sup 91]Zr atoms to an odd-parity E[sub 1] energy level in the range of 16000--19000 cm[sup [minus]1], are irradiated by a laser beam having a wavelength [lambda][sub 2] to raise the atoms from an E[sub l] level to an even-parity E[sub 2] energy level in the range of 35000--37000 cm[sup [minus]1] and are irradiated by a laser beam having a wavelength [lambda][sub 3] to cause a resonant transition of atoms from an E[sub 2] level to an autoionizing level above 53506 cm[sup [minus]1][lambda][sub 3] wavelengths of 5607, 6511 or 5756 [angstrom] will excite a zirconium atom from an E[sub 2] energy state of 36344 cm[sup [minus]1] to an autoionizing level; a [lambda][sub 3] wavelength of 5666 [angstrom] will cause an autoionizing transition from an E[sub 2] level of 36068 cm[sup [minus]1]; and a [lambda][sub 3] wavelength of 5662 [angstrom] will cause an ionizing resonance of an atom at an E[sub 2] level of 35904 cm[sup [minus]1]. 4 figures.
NASA Astrophysics Data System (ADS)
Qian, Jie; Cheng, Wei; Cao, Zhaoyuan; Chen, Xinjian; Mo, Jianhua
2017-02-01
Phase-resolved Doppler optical coherence tomography (PR-D-OCT) is a functional OCT imaging technique that can provide high-speed and high-resolution depth-resolved measurement on flow in biological materials. However, a common problem with conventional PR-D-OCT is that this technique often measures the flow motion projected onto the OCT beam path. In other words, it needs the projection angle to extract the absolute velocity from PR-D-OCT measurement. In this paper, we proposed a novel dual-beam PR-D-OCT method to measure absolute flow velocity without separate measurement on the projection angle. Two parallel light beams are created in sample arm and focused into the sample at two different incident angles. The images produced by these two beams are encoded to different depths in single B-scan. Then the Doppler signals picked up by the two beams together with the incident angle difference can be used to calculate the absolute velocity. We validated our approach in vitro on an artificial flow phantom with our home-built 1060 nm swept source OCT. Experimental results demonstrated that our method can provide an accurate measurement of absolute flow velocity with independency on the projection angle.
NASA Astrophysics Data System (ADS)
Dong, J. T.; Ji, F.; Xia, H. J.; Liu, Z. J.; Zhang, T. D.; Yang, L.
2018-01-01
An angle-resolved spectral Fabry-Pérot interferometer is reported for fast and accurate measurement of the refractive index dispersion of optical materials with parallel plate shape. The light sheet from the wavelength tunable laser is incident on the parallel plate with converging angles. The transmitted interference light for each angle is dispersed and captured by a 2D sensor, in which the rows and the columns are used to simultaneously record the intensities as a function of wavelength and incident angle, respectively. The interferogram, named angle-resolved spectral intensity distribution, is analyzed by fitting the phase information instead of finding the fringe peak locations that present periodic ambiguity. The refractive index dispersion and the physical thickness can be then retrieved from a single-shot interferogram within 18 s. Experimental results of an optical substrate standard indicate that the accuracy of the refractive index dispersion is less than 2.5 × 10-5 and the relative uncertainty of the thickness is 6 × 10-5 mm (3σ) due to the high stability and the single-shot measurement of the proposed system.
Autoionizing states driven by stochastic electromagnetic fields
NASA Astrophysics Data System (ADS)
Mouloudakis, G.; Lambropoulos, P.
2018-01-01
We have examined the profile of an isolated autoionizing resonance driven by a pulse of short duration and moderately strong field. The analysis has been based on stochastic differential equations governing the time evolution of the density matrix under a stochastic field. Having focused our quantitative analysis on the 2{{s}}2{{p}}({}1{{P}}) resonance of helium, we have investigated the role of field fluctuations and of the duration of the pulse. We report surprisingly strong distortion of the profile, even for peak intensity below the strong field limit. Our results demonstrate the intricate connection between intensity and pulse duration, with the latter appearing to be the determining influence, even for a seemingly short pulse of 50 fs. Further effects that would arise under much shorter pulses are discussed.
Constraining Aerosol Properties with the Spectrally-Resolved Phase Function of Pluto's Hazes
NASA Astrophysics Data System (ADS)
Parker, A. H.; Howett, C.; Olkin, C.; Protopapa, S.; Grundy, W. M.; Gladstone, R.; Young, L. A.; Horst, S. M.; Weaver, H. A., Jr.; Moore, J. M.; Ennico Smith, K.; Stern, A.
2017-12-01
The Multi-spectral Visible Imaging Camera (MVIC) and Lisa Hardaway Infrared Mapping Spectrometer (LEISA) aboard New Horizons imaged Pluto at high phase throughout departure from the system in July of 2015. The repeated MVIC color scans captured the phase behavior of Pluto's atmospheric hazes through phase angles of 165.0 to 169.5 degrees in four bandpasses in the visible and NIR. A spatially-resolved departure LEISA scan delivered moderate SNR NIR spectra of the hazes over wavelengths from 1.25 - 2.5 microns. Here we present our analysis of the departure MVIC and LEISA data, extracting high precision color phase curves of the hazes using the most up-to-date radiometric calibration and NIR gain drift corrections. We interpret these phase curves and spectra using Mie theory to constrain the size and composition of haze particles, with results indicating broad similarity to Titan aerosol analogues ("tholins"). Finally, we will explore the implications of the nature of these haze particles for the evolution of Pluto's surface as they settle out onto it over time.
Electronic structure of YbB 6 : Is it a topological insulator or not?
Kang, Chang -Jong; Denlinger, J. D.; Allen, J. W.; ...
2016-03-17
Here, to finally resolve the controversial issue of whether or not the electronic structure of YbB6 is nontrivially topological, we have made a combined study using angle-resolved photoemission spectroscopy (ARPES) of the nonpolar (110) surface and density functional theory (DFT). The flat-band conditions of the (110) ARPES avoid the strong band bending effects of the polar (001) surface and definitively show that YbB 6 has a topologically trivial B 2p–Yb 5d semiconductor band gap of ~0.3 eV. Accurate determination of the low energy band topology in DFT requires the use of a modified Becke-Johnson exchange potential incorporating spin-orbit coupling andmore » an on-site Yb 4f Coulomb interaction U as large as 7 eV. The DFT result, confirmed by a more precise GW band calculation, is similar to that of a small gap non-Kondo nontopological semiconductor. Additionally, the pressure-dependent electronic structure of YbB 6 is investigated theoretically and found to transform into a p–d overlap semimetal with small Yb mixed valency.« less
Universal precision sine bar attachment
NASA Technical Reports Server (NTRS)
Mann, Franklin D. (Inventor)
1989-01-01
This invention relates to an attachment for a sine bar which can be used to perform measurements during lathe operations or other types of machining operations. The attachment can be used for setting precision angles on vises, dividing heads, rotary tables and angle plates. It can also be used in the inspection of machined parts, when close tolerances are required, and in the layout of precision hardware. The novelty of the invention is believed to reside in a specific versatile sine bar attachment for measuring a variety of angles on a number of different types of equipment.
Angle-resolved molecular beam scattering of NO at the gas-liquid interface.
Zutz, Amelia; Nesbitt, David J
2017-08-07
This study presents first results on angle-resolved, inelastic collision dynamics of thermal and hyperthermal molecular beams of NO at gas-liquid interfaces. Specifically, a collimated incident beam of supersonically cooled NO ( 2 Π 1/2 , J = 0.5) is directed toward a series of low vapor pressure liquid surfaces ([bmim][Tf 2 N], squalane, and PFPE) at θ inc = 45(1)°, with the scattered molecules detected with quantum state resolution over a series of final angles (θ s = -60°, -30°, 0°, 30°, 45°, and 60°) via spatially filtered laser induced fluorescence. At low collision energies [E inc = 2.7(9) kcal/mol], the angle-resolved quantum state distributions reveal (i) cos(θ s ) probabilities for the scattered NO and (ii) electronic/rotational temperatures independent of final angle (θ s ), in support of a simple physical picture of angle independent sticking coefficients and all incident NO thermally accommodating on the surface. However, the observed electronic/rotational temperatures for NO scattering reveal cooling below the surface temperature (T elec < T rot < T S ) for all three liquids, indicating a significant dependence of the sticking coefficient on NO internal quantum state. Angle-resolved scattering at high collision energies [E inc = 20(2) kcal/mol] has also been explored, for which the NO scattering populations reveal angle-dependent dynamical branching between thermal desorption and impulsive scattering (IS) pathways that depend strongly on θ s . Characterization of the data in terms of the final angle, rotational state, spin-orbit electronic state, collision energy, and liquid permit new correlations to be revealed and investigated in detail. For example, the IS rotational distributions reveal an enhanced propensity for higher J/spin-orbit excited states scattered into near specular angles and thus hotter rotational/electronic distributions measured in the forward scattering direction. Even more surprisingly, the average NO scattering angle (⟨θ s ⟩) exhibits a remarkably strong correlation with final angular momentum, N, which implies a linear scaling between net forward scattering propensity and torque delivered to the NO projectile by the gas-liquid interface.
Angle-resolved molecular beam scattering of NO at the gas-liquid interface
NASA Astrophysics Data System (ADS)
Zutz, Amelia; Nesbitt, David J.
2017-08-01
This study presents first results on angle-resolved, inelastic collision dynamics of thermal and hyperthermal molecular beams of NO at gas-liquid interfaces. Specifically, a collimated incident beam of supersonically cooled NO (2 Π 1/2, J = 0.5) is directed toward a series of low vapor pressure liquid surfaces ([bmim][Tf2N], squalane, and PFPE) at θinc = 45(1)°, with the scattered molecules detected with quantum state resolution over a series of final angles (θs = -60°, -30°, 0°, 30°, 45°, and 60°) via spatially filtered laser induced fluorescence. At low collision energies [Einc = 2.7(9) kcal/mol], the angle-resolved quantum state distributions reveal (i) cos(θs) probabilities for the scattered NO and (ii) electronic/rotational temperatures independent of final angle (θs), in support of a simple physical picture of angle independent sticking coefficients and all incident NO thermally accommodating on the surface. However, the observed electronic/rotational temperatures for NO scattering reveal cooling below the surface temperature (Telec < Trot < TS) for all three liquids, indicating a significant dependence of the sticking coefficient on NO internal quantum state. Angle-resolved scattering at high collision energies [Einc = 20(2) kcal/mol] has also been explored, for which the NO scattering populations reveal angle-dependent dynamical branching between thermal desorption and impulsive scattering (IS) pathways that depend strongly on θs. Characterization of the data in terms of the final angle, rotational state, spin-orbit electronic state, collision energy, and liquid permit new correlations to be revealed and investigated in detail. For example, the IS rotational distributions reveal an enhanced propensity for higher J/spin-orbit excited states scattered into near specular angles and thus hotter rotational/electronic distributions measured in the forward scattering direction. Even more surprisingly, the average NO scattering angle (⟨θs⟩) exhibits a remarkably strong correlation with final angular momentum, N, which implies a linear scaling between net forward scattering propensity and torque delivered to the NO projectile by the gas-liquid interface.
NASA Astrophysics Data System (ADS)
Braun, Jürgen; Minár, Ján; Ebert, Hubert
2018-04-01
Various apparative developments extended the potential of angle-resolved photoemission spectroscopy tremendously during the last two decades. Modern experimental arrangements consisting of new photon sources, analyzers and detectors supply not only extremely high angle and energy resolution but also spin resolution. This provides an adequate platform to study in detail new materials like low-dimensional magnetic structures, Rashba systems, topological insulator materials or high TC superconductors. The interest in such systems has grown enormously not only because of their technological relevance but even more because of exciting new physics. Furthermore, the use of photon energies from few eV up to several keV makes this experimental technique a rather unique tool to investigate the electronic properties of solids and surfaces. The following article reviews the corresponding recent theoretical developments in the field of angle-resolved photoemission with a special emphasis on correlation effects, temperature and relativistic aspects. The most successful theoretical approach to deal with angle-resolved photoemission is the so-called spectral function or one-step formulation of the photoemission process. Nowadays, the one-step model allows for photocurrent calculations for photon energies ranging from a few eV to more than 10 keV, to deal with arbitrarily ordered and disordered systems, to account for finite temperatures, and considering in addition strong correlation effects within the dynamical mean-field theory or similar advanced approaches.
NASA Astrophysics Data System (ADS)
Ogawa, Manami; Yamamoto, Susumu; Kousa, Yuka; Nakamura, Fumitaka; Yukawa, Ryu; Fukushima, Akiko; Harasawa, Ayumi; Kondoh, Hiroshi; Tanaka, Yoshihito; Kakizaki, Akito; Matsuda, Iwao
2012-02-01
We have developed a soft x-ray time-resolved photoemission spectroscopy system using synchrotron radiation (SR) at SPring-8 BL07LSU and an ultrashort pulse laser system. Two-dimensional angle-resolved measurements were performed with a time-of-flight-type analyzer. The photoemission spectroscopy system is synchronized to light pulses of SR and laser using a time control unit. The performance of the instrument is demonstrated by mapping the band structure of a Si(111) crystal over the surface Brillouin zones and observing relaxation of the surface photo-voltage effect using the pump (laser) and probe (SR) method.
Ogawa, Manami; Yamamoto, Susumu; Kousa, Yuka; Nakamura, Fumitaka; Yukawa, Ryu; Fukushima, Akiko; Harasawa, Ayumi; Kondoh, Hiroshi; Tanaka, Yoshihito; Kakizaki, Akito; Matsuda, Iwao
2012-02-01
We have developed a soft x-ray time-resolved photoemission spectroscopy system using synchrotron radiation (SR) at SPring-8 BL07LSU and an ultrashort pulse laser system. Two-dimensional angle-resolved measurements were performed with a time-of-flight-type analyzer. The photoemission spectroscopy system is synchronized to light pulses of SR and laser using a time control unit. The performance of the instrument is demonstrated by mapping the band structure of a Si(111) crystal over the surface Brillouin zones and observing relaxation of the surface photo-voltage effect using the pump (laser) and probe (SR) method.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Xie, Min; Shen, Zhitao; Pratt, S. T.
Vibrational autoionization of Rydberg states provides key information about nonadiabatic processes above an ionization threshold. In this work, we employed time-of-flight mass detection of CH 3SH + to record vibrational-state selective photo-ionization efficiency (PIE) spectra of jet-cooled methanethiol (CH 3SH) on exciting CH 3SH to a specific vibrationally excited state with an infrared (IR) laser, followed by excitation with a tunable laser in the vacuum-ultraviolet (VUV) region for ionization. Autoionizing Rydberg states assigned to the ns, np, nd and nf series are identified. When IR light at 2601 (ν 3, SH stretching mode) and 2948 cm -1 (ν 2, CHmore » 3 symmetric stretching mode) was employed, the Rydberg series converged to the respective vibrationally excited (ν 3 and ν 2) states of CH 3SH +. When IR light at 3014 cm -1 (overlapped ν 1/ν 9, CH 3 antisymmetric stretching and CH 2 antisymmetric stretching modes) was employed, Rydberg series converging to two vibrationally excited states (ν 1 and ν 9) of CH 3SH + were observed. When IR light at 2867 cm -1 (2ν 10, overtone of CH 3 deformation mode) and 2892 cm -1 (2ν 4, overtone of CH 2 scissoring mode) was employed, both Δν = -1 and Δν = -2 ionization transitions were observed; there is evidence for direct ionization from the initial state into the CH 3SH + (ν 4 + = 1) continuum. In all observed IR-VUV-PIE spectra, the ns and nd series show intensity greater than the other Rydberg series, which is consistent with the fact that the highest-occupied molecular orbital of CH 3SH is a p-like lone pair orbital on the S atom. Finally, the quantum yields for autoionization of various vibrational excited states are discussed. Values of ν 1 = 3035, ν 2 = 2884, ν 3 = 2514, and ν 9 = 2936 cm -1 for CH 3SH + derived from the converged limits agree satisfactorily with values observed for Ar-tagged CH 3SH + at 3026, 2879, 2502, and 2933 cm -1.« less
NASA Astrophysics Data System (ADS)
Marante, Carlos; Klinker, Markus; Kjellsson, Tor; Lindroth, Eva; González-Vázquez, Jesús; Argenti, Luca; Martín, Fernando
2017-08-01
The XCHEM approach interfaces well established quantum chemistry packages with scattering numerical methods in order to describe single-ionization processes in atoms and molecules. This should allow one to describe electron correlation in the continuum at the same level of accuracy as quantum chemistry methods do for bound states. Here we have applied this method to study multichannel photoionization of Ne in the vicinity of the autoionizing states lying between the 2 s22 p5 and 2 s 2 p6 ionization thresholds. The calculated total photoionization cross sections are in very good agreement with the absolute measurement of Samson et al. [J. Electron Spectrosc. Relat. Phenom. 123, 265 (2002), 10.1016/S0368-2048(02)00026-9], and with independent benchmark calculations performed at the same level of theory. From these cross sections, we have extracted resonance positions, total autoionization widths, Fano profile parameters, and correlation parameters for the lowest three autoionizing states. The values of these parameters are in good agreement with those reported in earlier theoretical and experimental work. We have also evaluated β asymmetry parameter and partial photoionization cross sections and, from the latter, partial autoionization widths and Starace parameters for the same resonances, not yet available in the literature. Resonant features in the calculated β parameter are in good agreement with the experimental observations. We have found that the three lowest resonances preferentially decay into the 2 p-1ɛ d continuum rather than into the 2 p-1ɛ s one [Phys. Rev. A 89, 043415 (2014), 10.1103/PhysRevA.89.043415], in agreement with previous expectations, and that in the vicinity of the resonances the partial 2 p-1ɛ s cross section can be larger than the 2 p-1ɛ d one, in contrast with the accepted idea that the latter should amply dominate in the whole energy range. These results show the potential of the XCHEM approach to describe highly correlated process in the ionization continuum of many-electron systems, in particular molecules, for which the XCHEM code has been specifically designed.
Xie, Min; Shen, Zhitao; Pratt, S. T.; ...
2017-10-24
Vibrational autoionization of Rydberg states provides key information about nonadiabatic processes above an ionization threshold. In this work, we employed time-of-flight mass detection of CH 3SH + to record vibrational-state selective photo-ionization efficiency (PIE) spectra of jet-cooled methanethiol (CH 3SH) on exciting CH 3SH to a specific vibrationally excited state with an infrared (IR) laser, followed by excitation with a tunable laser in the vacuum-ultraviolet (VUV) region for ionization. Autoionizing Rydberg states assigned to the ns, np, nd and nf series are identified. When IR light at 2601 (ν 3, SH stretching mode) and 2948 cm -1 (ν 2, CHmore » 3 symmetric stretching mode) was employed, the Rydberg series converged to the respective vibrationally excited (ν 3 and ν 2) states of CH 3SH +. When IR light at 3014 cm -1 (overlapped ν 1/ν 9, CH 3 antisymmetric stretching and CH 2 antisymmetric stretching modes) was employed, Rydberg series converging to two vibrationally excited states (ν 1 and ν 9) of CH 3SH + were observed. When IR light at 2867 cm -1 (2ν 10, overtone of CH 3 deformation mode) and 2892 cm -1 (2ν 4, overtone of CH 2 scissoring mode) was employed, both Δν = -1 and Δν = -2 ionization transitions were observed; there is evidence for direct ionization from the initial state into the CH 3SH + (ν 4 + = 1) continuum. In all observed IR-VUV-PIE spectra, the ns and nd series show intensity greater than the other Rydberg series, which is consistent with the fact that the highest-occupied molecular orbital of CH 3SH is a p-like lone pair orbital on the S atom. Finally, the quantum yields for autoionization of various vibrational excited states are discussed. Values of ν 1 = 3035, ν 2 = 2884, ν 3 = 2514, and ν 9 = 2936 cm -1 for CH 3SH + derived from the converged limits agree satisfactorily with values observed for Ar-tagged CH 3SH + at 3026, 2879, 2502, and 2933 cm -1.« less
Hart, Alister J; Skinner, John A; Henckel, Johann; Sampson, Barry; Gordon, Fabiana
2011-09-01
Many factors affect the blood metal ion levels after metal-on-metal (MOM) hip arthroplasty. The main surgically adjustable variable is the amount of coverage of the head provided by the cup which is a function of the inclination and version angles. However, most studies have used plain radiographs which have questionable precision and accuracy, particularly for version and large diameter metal heads; further, these studies do not simultaneously assess version and inclination. Thus the relationship between version and blood metal ions levels has not been resolved. We determined whether cup inclination and version influence blood metal ion levels while adjusting for age at assessment, gender, body mass index, horizontal femoral offset, head size, manufacturer hip type, and Oxford hip score. We prospectively followed 100 individuals (51 females, 49 males) with unilateral MOM hip resurfacing who underwent clinical assessment, CT scanning, and blood metal ion measurement. Multiple regression analysis was used to determine which variables were predictors of blood metal ion levels and to model the effect of these variables. Only cup inclination, version angles, and gender influenced blood cobalt or chromium levels. Cobalt and chromium levels positively correlated with inclination angle and negatively correlated with version angle. The effect of changes in version angle was less than for inclination angle. Based on our observations, we developed a formula to predict the effect of these parameters on metal ion levels. Our data suggest insufficient cup version can cause high blood metal ions after MOM hip arthroplasty. We were unable to show that excessive version caused high levels. Level II, prognostic study. See Guidelines for Authors for a complete description of levels of evidence.
Binary collision model for neon Auger spectra from neon ion bombardment of the aluminum surface
NASA Technical Reports Server (NTRS)
Pepper, S. V.
1986-01-01
A model is developed to account for the angle-resolved Auger spectra from neon ion bombardment of the aluminum surface recently obtained by Pepper and Aron. The neon is assumed to be excited in a single asymmetric neon-aluminum-collision and scattered back into the vacuum where it emits an Auger electron. The velocity of the Auger electron acquires a Doppler shift by virtue of the emission from a moving source. The dependence of the Auger peak shape and energy on the incident ion energy, angle of incidence and on the angle of Auger electron emission with respect to the surface is presented. Satisfactory agreement with the angle resolved experimental observations is obtained. The dependence of the angle-integrated Auger yield on the incident ion energy and angle of incidence is also obtained and shown to be in satisfactory agreement with available experimental evidence.
An innovative Yb-based ultrafast deep ultraviolet source for time-resolved photoemission experiments
DOE Office of Scientific and Technical Information (OSTI.GOV)
Boschini, F.; Hedayat, H.; Dallera, C.
2014-12-15
Time- and angle-resolved photoemission spectroscopy is a powerful technique to study ultrafast electronic dynamics in solids. Here, an innovative optical setup based on a 100-kHz Yb laser source is presented. Exploiting non-collinear optical parametric amplification and sum-frequency generation, ultrashort pump (hν = 1.82 eV) and ultraviolet probe (hν = 6.05 eV) pulses are generated. Overall temporal and instrumental energy resolutions of, respectively, 85 fs and 50 meV are obtained. Time- and angle-resolved measurements on BiTeI semiconductor are presented to show the capabilities of the setup.
Wang, Zhiming; Zhong, Z.; Walker, S. McKeown; ...
2017-03-10
Engineering the electronic band structure of two-dimensional electron liquids (2DELs) confined at the surface or interface of transition metal oxides is key to unlocking their full potential. Here we describe a new approach to tailoring the electronic structure of an oxide surface 2DEL demonstrating the lateral modulation of electronic states with atomic scale precision on an unprecedented length scale comparable to the Fermi wavelength. To this end, we use pulsed laser deposition to grow anatase TiO 2 films terminated by a (1 x 4) in-plane surface reconstruction. Employing photo-stimulated chemical surface doping we induce 2DELs with tunable carrier densities thatmore » are confined within a few TiO 2 layers below the surface. Subsequent in situ angle resolved photoemission experiments demonstrate that the (1 x 4) surface reconstruction provides a periodic lateral perturbation of the electron liquid. Furthermore, this causes strong backfolding of the electronic bands, opening of unidirectional gaps and a saddle point singularity in the density of states near the chemical potential.« less
Study on manufacturing method of optical surface with high precision in angle and surface
NASA Astrophysics Data System (ADS)
Yu, Xin; Li, Xin; Yu, Ze; Zhao, Bin; Zhang, Xuebin; Sun, Lipeng; Tong, Yi
2016-10-01
This paper studied a manufacturing processing of optical surface with high precision in angel and surface. By theoretical analysis of the relationships between the angel precision and surface, the measurement conversion of the technical indicators, optical-cement method application, the optical-cement tooling design, the experiment has been finished successfully, the processing method has been verified, which can be also used in the manufacturing of the optical surface with similar high precision in angle and surface.
Bok, Jin Mo; Bae, Jong Ju; Choi, Han-Yong; Varma, Chandra M.; Zhang, Wentao; He, Junfeng; Zhang, Yuxiao; Yu, Li; Zhou, X. J.
2016-01-01
A profound problem in modern condensed matter physics is discovering and understanding the nature of fluctuations and their coupling to fermions in cuprates, which lead to high-temperature superconductivity and the invariably associated strange metal state. We report the quantitative determination of normal and pairing self-energies, made possible by laser-based angle-resolved photoemission measurements of unprecedented accuracy and stability. Through a precise inversion procedure, both the effective interactions in the attractive d-wave symmetry and the repulsive part in the full symmetry are determined. The latter is nearly angle-independent. Near Tc, both interactions are nearly independent of frequency and have almost the same magnitude over the complete energy range of up to about 0.4 eV, except for a low-energy feature at around 50 meV that is present only in the repulsive part, which has less than 10% of the total spectral weight. Well below Tc, they both change similarly, with superconductivity-induced features at low energies. Besides finding the pairing self-energy and the attractive interactions for the first time, these results expose the central paradox of the problem of high Tc: how the same frequency-independent fluctuations can dominantly scatter at angles ±π/2 in the attractive channel to give d-wave pairing and lead to angle-independent repulsive scattering. The experimental results are compared with available theoretical calculations based on antiferromagnetic fluctuations, the Hubbard model, and quantum-critical fluctuations of the loop-current order. PMID:26973872
Angle-resolved effective potentials for disk-shaped molecules
NASA Astrophysics Data System (ADS)
Heinemann, Thomas; Palczynski, Karol; Dzubiella, Joachim; Klapp, Sabine H. L.
2014-12-01
We present an approach for calculating coarse-grained angle-resolved effective pair potentials for uniaxial molecules. For integrating out the intramolecular degrees of freedom we apply umbrella sampling and steered dynamics techniques in atomistically-resolved molecular dynamics (MD) computer simulations. Throughout this study we focus on disk-like molecules such as coronene. To develop the methods we focus on integrating out the van der Waals and intramolecular interactions, while electrostatic charge contributions are neglected. The resulting coarse-grained pair potential reveals a strong temperature and angle dependence. In the next step we fit the numerical data with various Gay-Berne-like potentials to be used in more efficient simulations on larger scales. The quality of the resulting coarse-grained results is evaluated by comparing their pair and many-body structure as well as some thermodynamic quantities self-consistently to the outcome of atomistic MD simulations of many-particle systems. We find that angle-resolved potentials are essential not only to accurately describe crystal structures but also for fluid systems where simple isotropic potentials start to fail already for low to moderate packing fractions. Further, in describing these states it is crucial to take into account the pronounced temperature dependence arising in selected pair configurations due to bending fluctuations.
Precision controllability of the F-15 airplane
NASA Technical Reports Server (NTRS)
Sisk, T. R.; Matheny, N. W.
1979-01-01
A flying qualities evaluation conducted on a preproduction F-15 airplane permitted an assessment to be made of its precision controllability in the high subsonic and low transonic flight regime over the allowable angle of attack range. Precision controllability, or gunsight tracking, studies were conducted in windup turn maneuvers with the gunsight in the caged pipper mode and depressed 70 mils. This evaluation showed the F-15 airplane to experience severe buffet and mild-to-moderate wing rock at the higher angles of attack. It showed the F-15 airplane radial tracking precision to vary from approximately 6 to 20 mils over the load factor range tested. Tracking in the presence of wing rock essentially doubled the radial tracking error generated at the lower angles of attack. The stability augmentation system affected the tracking precision of the F-15 airplane more than it did that of previous aircraft studied.
NASA Astrophysics Data System (ADS)
Kadlubowski, S.; Sawicki, P.; Sowinski, S.; Rokita, B.; Bures, K. D.; Rosiak, J. M.; Ulanski, P.
2018-01-01
Time-resolved pulse radiolysis, utilizing short pulses of high-energy electrons from accelerators, is an effective method for rapidly generating free radicals and other transient species in solution. Combined with fast time-resolved spectroscopic detection (typically in the ultraviolet/visible/near-infrared), it is invaluable for monitoring the reactivity of species subjected to radiolysis on timescales ranging from picoseconds to seconds. When used for polymer solutions, pulse radiolysis can be coupled with light-scattering detection, creating a powerful tool for kinetic and mechanistic analysis of processes like degradation or cross-linking of macromolecules. Changes in the light scattering intensity (LSI) of polymer solutions are indicative of alterations in the molecular weight and/or in the radius of gyration, i.e., the dimensions and shape of the macromolecules. In addition to other detection methods, LSI technique provides a convenient tool to study radiation-induced alterations in macromolecules as a function of time after the pulse. Pulse radiolysis systems employing this detection mode have been so far constructed to follow light scattered at a single angle (typically the right angle) to the incident light beam. Here we present an advanced pulse radiolysis & multi-angle light-scattering-intensity system (PR-MALLS) that has been built at IARC and is currently in the phase of optimization and testing. Idea of its design and operation is described and preliminary results for radiation-induced degradation of pullulan as well as polymerization and crosslinking of poly(ethylene glycol) diacrylate are presented. Implementation of the proposed system provides a novel research tool, which is expected to contribute to the expansion of knowledge on free-radical reactions in monomer- and polymer solutions, by delivering precise kinetic data on changes in molecular weight and size, and thus allowing to formulate or verify reaction mechanisms. The proposed method is universal and can be applied for studying both natural and synthetic polymers. The developed system can be also valuable in studies of the border of biology and medicine, especially on radical reactions of biopolymers and their conformational transitions. Furthermore, capability to follow fast changes in mass and dimensions of nanobjects may be of significant importance for nanoscience and nanotechnology.
NASA Astrophysics Data System (ADS)
Keqi, A.; Gehlmann, M.; Conti, G.; Nemšák, S.; Rattanachata, A.; Minár, J.; Plucinski, L.; Rault, J. E.; Rueff, J. P.; Scarpulla, M.; Hategan, M.; Pálsson, G. K.; Conlon, C.; Eiteneer, D.; Saw, A. Y.; Gray, A. X.; Kobayashi, K.; Ueda, S.; Dubon, O. D.; Schneider, C. M.; Fadley, C. S.
2018-04-01
We have investigated the electronic structure of the dilute magnetic semiconductor (DMS) G a0.98M n0.02P and compared it to that of an undoped GaP reference sample, using hard x-ray photoelectron spectroscopy (HXPS) and hard x-ray angle-resolved photoemission spectroscopy (HARPES) at energies of about 3 keV. We present experimental data, as well as theoretical calculations, to understand the role of the Mn dopant in the emergence of ferromagnetism in this material. Both core-level spectra and angle-resolved or angle-integrated valence spectra are discussed. In particular, the HARPES experimental data are compared to free-electron final-state model calculations and to more accurate one-step photoemission theory. The experimental results show differences between G a0.98M n0.02P and GaP in both angle-resolved and angle-integrated valence spectra. The G a0.98M n0.02P bands are broadened due to the presence of Mn impurities that disturb the long-range translational order of the host GaP crystal. Mn-induced changes of the electronic structure are observed over the entire valence band range, including the presence of a distinct impurity band close to the valence-band maximum of the DMS. These experimental results are in good agreement with the one-step photoemission calculations and a prior HARPES study of G a0.97M n0.03As and GaAs [Gray et al., Nat. Mater. 11, 957 (2012), 10.1038/nmat3450], demonstrating the strong similarity between these two materials. The Mn 2 p and 3 s core-level spectra also reveal an essentially identical state in doping both GaAs and GaP.
Precision in the perception of direction of a moving pattern
NASA Technical Reports Server (NTRS)
Stone, Leland S.
1988-01-01
The precision of the model of pattern motion analysis put forth by Adelson and Movshon (1982) who proposed that humans determine the direction of a moving plaid (the sum of two sinusoidal gratings of different orientations) in two steps is qualitatively examined. The volocities of the grating components are first estimated, then combined using the intersection of constraints to determine the velocity of the plaid as a whole. Under the additional assumption that the noise sources for the component velocities are independent, an approximate expression can be derived for the precision in plaid direction as a function of the precision in the speed and direction of the components. Monte Carlo simulations verify that the expression is valid to within 5 percent over the natural range of the parameters. The expression is then used to predict human performance based on available estimates of human precision in the judgment of single component speed. Human performance is predicted to deteriorate by a factor of 3 as half the angle between the wavefronts (theta) decreases from 60 to 30 deg, but actual performance does not. The mean direction discrimination for three human observers was 4.3 plus or minus 0.9 deg (SD) for theta = 60 deg and 5.9 plus or minus 1.2 for theta = 30 deg. This discrepancy can be resolved in two ways. If the noises in the internal representations of the component speeds are smaller than the available estimates or if these noises are not independent, then the psychophysical results are consistent with the Adelson-Movshon hypothesis.
Unsteady Transonic Flow Past Airfoils in Rigid Body Motion.
1981-03-01
coordinate system. Numerical experiments show that the scheme is very stable and is able to resolve the highly non- linear transonic effects for flutter...Numerical experiments show that the scheme is very stable and is able to resolve the highly nonlinear transonic effects for flutter analysis within...of attack, the angle between the flight direction and the airfoil chord. The effect of chanqinthe angle of attack of a conventional symmetric airfoil
NASA Astrophysics Data System (ADS)
Kostogryz, Nadiia; Berdyugina, Svetlana; Gisler, Daniel; Berkefeld, Thomas
2017-04-01
In planetary atmospheres, main sources of opacity are molecular absorption and scattering on molecules, hazes and aerosols. Hence, light reflected from a planetary atmosphere can be linearly polarized. Polarization study of inner solar system planets and exoplanets is a powerful method to characterize their atmospheres, because of a wide range of observable phase angles. For outer solar system planets, observable phase angles are very limited. For instance, Uranus can only be observed up to 3.2 degrees away from conjunctions, and its disk-integrated polarization is close to zero due to the back-scattering geometry. However, resolving the disk of Uranus and measuring the center-to-limb polarization can help constraining the vertical atmospheric structure and the nature of scattering aerosols and particles. In October 2016, we carried out polarization measurements of Uranus in narrow-band filters centered at methane bands and the adjacent continuum using the GREGOR Planet Polarimeter (GPP). The GPP is a high-precision polarimeter and is mounted at the 1.5-m GREGOR solar telescope, which is suitable for observing at night. In order to reach a high spatial resolution, the instrument uses an adaptive-optics system of the telescope. To interpret our measurements, we solve the polarized radiative transfer problem taking into account different scattering and absorption opacities. We calculate the center-to-limb variation of polarization of Uranus' disk in the continuum spectrum and in methane bands. By varying the vertical distribution of haze and cloud layers, we derive the vertical structure of the best-fit Uranus atmosphere.
Scanning fiber angle-resolved low coherence interferometry
Zhu, Yizheng; Terry, Neil G.; Wax, Adam
2010-01-01
We present a fiber-optic probe for Fourier-domain angle-resolved low coherence interferometry for the determination of depth-resolved scatterer size. The probe employs a scanning single-mode fiber to collect the angular scattering distribution of the sample, which is analyzed using the Mie theory to obtain the average size of the scatterers. Depth sectioning is achieved with low coherence Mach–Zehnder interferometry. In the sample arm of the interferometer, a fixed fiber illuminates the sample through an imaging lens and a collection fiber samples the backscattered angular distribution by scanning across the Fourier plane image of the sample. We characterize the optical performance of the probe and demonstrate the ability to execute depth-resolved sizing with subwavelength accuracy by using a double-layer phantom containing two sizes of polystyrene microspheres. PMID:19838271
Measuring Speed Of Rotation With Two Brushless Resolvers
NASA Technical Reports Server (NTRS)
Howard, David E.
1995-01-01
Speed of rotation of shaft measured by use of two brushless shaft-angle resolvers aligned so electrically and mechanically in phase with each other. Resolvers and associated circuits generate voltage proportional to speed of rotation (omega) in both magnitude and sign. Measurement principle exploits simple trigonometric identity.
LaForge, A. C.; Drabbels, M.; Brauer, N. B.; Coreno, M.; Devetta, M.; Di Fraia, M.; Finetti, P.; Grazioli, C.; Katzy, R.; Lyamayev, V.; Mazza, T.; Mudrich, M.; O'Keeffe, P.; Ovcharenko, Y.; Piseri, P.; Plekan, O.; Prince, K. C.; Richter, R.; Stranges, S.; Callegari, C.; Möller, T.; Stienkemeier, F.
2014-01-01
Free electron lasers (FELs) offer the unprecedented capability to study reaction dynamics and image the structure of complex systems. When multiple photons are absorbed in complex systems, a plasma-like state is formed where many atoms are ionized on a femtosecond timescale. If multiphoton absorption is resonantly-enhanced, the system becomes electronically-excited prior to plasma formation, with subsequent decay paths which have been scarcely investigated to date. Here, we show using helium nanodroplets as an example that these systems can decay by a new type of process, named collective autoionization. In addition, we show that this process is surprisingly efficient, leading to ion abundances much greater than that of direct single-photon ionization. This novel collective ionization process is expected to be important in many other complex systems, e.g. macromolecules and nanoparticles, exposed to high intensity radiation fields. PMID:24406316
DOE Office of Scientific and Technical Information (OSTI.GOV)
Liu, Yuan; Gottwald, T.; Mattolat, C.
We obtained multi-step resonance ionization spectroscopy of cobalt using a hot-cavity laser ion source and three Ti:Sapphire lasers. Furthermore, the photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d 74s5s h 4F 9/2, 3d 74s4d f 4G 11/2, and 3d 74s4d f 4H 13/2 and converge to the first four excited states of singly ionized Co. Our analyses of the Rydberg series yield 63564.689 0.036 cm -1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonancemore » ionization scheme that employs an autoinizing Rydberg state in the last transition, we obtained an overall ionization efficiency of about 18% for Co.« less
Liu, Yuan; Gottwald, T.; Mattolat, C.; ...
2017-03-20
We obtained multi-step resonance ionization spectroscopy of cobalt using a hot-cavity laser ion source and three Ti:Sapphire lasers. Furthermore, the photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d 74s5s h 4F 9/2, 3d 74s4d f 4G 11/2, and 3d 74s4d f 4H 13/2 and converge to the first four excited states of singly ionized Co. Our analyses of the Rydberg series yield 63564.689 0.036 cm -1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonancemore » ionization scheme that employs an autoinizing Rydberg state in the last transition, we obtained an overall ionization efficiency of about 18% for Co.« less
Absolute partial photoionization cross sections of ethylene
NASA Astrophysics Data System (ADS)
Grimm, F. A.; Whitley, T. A.; Keller, P. R.; Taylor, J. W.
1991-07-01
Absolute partial photoionization cross sections for ionization out of the first four valence orbitals to the X 2B 3u, A 2B 3g, B 2A g and C 2B 2u states of the C 2H 4+ ion are presented as a function of photon energy over the energy range from 12 to 26 eV. The experimental results have been compared to previously published relative partial cross sections for the first two bands at 18, 21 and 24 eV. Comparison of the experimental data with continuum multiple scattering Xα calculations provides evidence for extensive autoionization to the X 2B 3u state and confirms the predicted shape resonances in ionization to the A 2B 3g and B 2A g states. Identification of possible transitions for the autoionizing resonances have been made using multiple scattering transition state calculations on Rydberg excited states.
Miller, C.M.; Nogar, N.S.
1982-09-02
Photoionization via autoionizing atomic levels combined with conventional mass spectroscopy provides a technique for quantitative analysis of trace quantities of chemical elements in the presence of much larger amounts of other elements with substantially the same atomic mass. Ytterbium samples smaller than 10 ng have been detected using an ArF* excimer laser which provides the atomic ions for a time-of-flight mass spectrometer. Elemental selectivity of greater than 5:1 with respect to lutetium impurity has been obtained. Autoionization via a single photon process permits greater photon utilization efficiency because of its greater absorption cross section than bound-free transitions, while maintaining sufficient spectroscopic structure to allow significant photoionization selectivity between different atomic species. Separation of atomic species from others of substantially the same atomic mass is also described.
Indirect double photoionization of water
NASA Astrophysics Data System (ADS)
Resccigno, T. N.; Sann, H.; Orel, A. E.; Dörner, R.
2011-05-01
The vertical double ionization thresholds of small molecules generally lie above the dissociation limits corresponding to formation of two singly charged fragments. This gives the possibility of populating singly charged molecular ions by photoionization in the Franck-Condon region at energies below the lowest dication state, but above the dissociation limit into two singly charged fragment ions. This process can produce a superexcited neutral fragment that autoionizes at large internuclear separation. We study this process in water, where absorption of a photon produces an inner-shell excited state of H2O+ that fragments to H++OH*. The angular distribution of secondary electrons produced by OH* when it autoionizes produces a characteristic asymmetric pattern that reveals the distance, and therefore the time, at which the decay takes place. LBNL, Berkeley, CA, J. W. Goethe Universität, Frankfurt, Germany. Work performed under auspices of US DOE and supported by OBES, Div. of Chemical Sciences.
High-Resolution Triple Resonance Autoionization of Uranium Isotopes
DOE Office of Scientific and Technical Information (OSTI.GOV)
Schumann, Philipp G.; Wendt, K; Bushaw, Bruce A.
2005-11-01
The near-threshold autoionization (AI) spectrum of uranium has been investigated by triple-resonance excitation with single-mode continuous lasers. Spectra were recorded over the first {approx}30 cm-1 above the first ionization limit at a resolution of 3x10-4 cm 1 using intermediate states with different J values (6, 7, 8) to assign AI level total angular momentum JAI = 5 to 9. Resonances with widths ranging from 8 MHz to 30 GHz were observed; the strongest ones have JAI = 9 and widths of {approx} 60 MHz. Hyperfine structures for 235U and isotope shifts for 234,235U have been measured in the two intermediatemore » levels and in the final AI level for the most favorable excitation path. These measurements were performed using aqueous samples containing sub-milligram quantities of uranium at natural isotopic abundances, indicating the potential of this approach for trace isotope ratio determinations.« less
First Results from the CHARA Array. V. Binary Star Astrometry: The Case of 12 Persei
NASA Astrophysics Data System (ADS)
Bagnuolo, William G., Jr.; Taylor, Stuart F.; McAlister, Harold A.; ten Brummelaar, Theo; Gies, Douglas R.; Ridgway, Stephen T.; Sturmann, Judit; Sturmann, Laszlo; Turner, Nils H.; Berger, David H.; Gudehus, Donald
2006-05-01
We have obtained high-resolution orbital data with the CHARA Array for the bright star 12 Persei, a resolved double-lined spectroscopic binary. We describe the data reduction process, which can give precision in separation of up to 25 μas along a given baseline. For this object we find a semimajor axis of a=53.18+/-0.15 mas, which is 0.3% smaller than that of Barlow and coworkers, but with much improved precision. The inclination angle i increases to 128.17d+/-0.14d, compared to 126.77d+/-0.56d of Barlow and coworkers, again with better precision. We also found an intensity ratio for the components in the K' band (λ=2.13 μm) of r=0.72+/-0.01, or ΔK'=0.409+/-0.013, after allowing for the partial resolution of the components. Assuming the spectral types of the components, we find that ΔV=0.51, as compared to 0.57 by Barlow and coworkers. The revised masses (Mp=1.382+/-0.019 and Ms=1.240+/-0.017 Msolar) are found to be 5.8% larger than those of Barlow and coworkers, and the components are thus even more overmassive. The overall accuracy in the masses is about 1.3%, now primarily limited by the spectroscopically determined radial velocities. The precision of the masses due to the interferometrically derived ``visual'' orbit alone is only about 0.2%.
Hussaini, Zahra; Lin, Pin Ann; Natarajan, Bharath; Zhu, Wenhui; Sharma, Renu
2018-03-01
For many reaction processes, such as catalysis, phase transformations, nanomaterial synthesis etc., nanoscale observations at high spatial (sub-nanometer) and temporal (millisecond) resolution are required to characterize and comprehend the underlying factors that favor one reaction over another. The combination of such spatial and temporal resolution (up to 600 µs), while rich in information, produces a large number of snapshots, each of which must be analyzed to obtain the structural (and thereby chemical) information. Here we present a methodology for automated quantitative measurement of real-time atomic position fluctuations in a nanoparticle. We leverage a combination of several image processing algorithms to precisely identify the positions of the atomic columns in each image. A geometric model is then used to measure the time-evolution of distances and angles between neighboring atomic columns to identify different phases and quantify local structural fluctuations. We apply this technique to determine the atomic-level fluctuations in the relative fractions of metal and metal-carbide phases in a cobalt catalyst nanoparticle during single-walled carbon nanotube (SWCNT) growth. These measurements provided a means to obtain the number of carbon atoms incorporated into and released from the catalyst particle, thereby helping resolve carbon reaction pathways during SWCNT growth. Further we demonstrate the use of this technique to measure the reaction kinetics of iron oxide reduction. Apart from reducing the data analysis time, the statistical approach allows us to measure atomic distances with sub-pixel resolution. We show that this method can be applied universally to measure atomic positions with a precision of 0.01 nm from any set of atomic-resolution video images. With the advent of high time-resolution direct detection cameras, we anticipate such methods will be essential in addressing the metrology problem of quantifying large datasets of time-resolved images in future. Published by Elsevier B.V.
Angle-resolved Auger electron spectra induced by neon ion impact on aluminum
NASA Technical Reports Server (NTRS)
Pepper, S. V.; Aron, P. R.
1986-01-01
Auger electron emission from aluminum bombarded with 1 to 5 keV neon ions was studied by angle-resolved electron spectroscopy. The position and shape of the spectral features depended on the incident ion energy, angle of ion incidence, and electron take-off angle with respect to the aluminum surface. These spectral dependencies were interpreted in terms of the Doppler shift given to the Auger electron velocity by the excited atom ejected into the vacuum. For oblique ion incidence it is concluded that a flux of high energy atoms are ejected in a direction close to the projection of the ion beam on the target surface. In addition, a new spectral feature was found and identified as due to Auger emission from excited neon in the aluminum matrix.
NASA Astrophysics Data System (ADS)
Jaroniec, Christopher P.; Macphee, Cait E.; Bajaj, Vikram S.; McMahon, Michael T.; Dobson, Christopher M.; Griffin, Robert G.
2004-01-01
Amyloid fibrils are self-assembled filamentous structures associated with protein deposition conditions including Alzheimer's disease and the transmissible spongiform encephalopathies. Despite the immense medical importance of amyloid fibrils, no atomic-resolution structures are available for these materials, because the intact fibrils are insoluble and do not form diffraction-quality 3D crystals. Here we report the high-resolution structure of a peptide fragment of the amyloidogenic protein transthyretin, TTR(105-115), in its fibrillar form, determined by magic angle spinning NMR spectroscopy. The structure resolves not only the backbone fold but also the precise conformation of the side chains. Nearly complete 13C and 15N resonance assignments for TTR(105-115) formed the basis for the extraction of a set of distance and dihedral angle restraints. A total of 76 self-consistent experimental measurements, including 41 restraints on 19 backbone dihedral angles and 35 13C-15N distances between 3 and 6 Å were obtained from 2D and 3D NMR spectra recorded on three fibril samples uniformly 13C, 15N-labeled in consecutive stretches of four amino acids and used to calculate an ensemble of peptide structures. Our results indicate that TTR(105-115) adopts an extended -strand conformation in the amyloid fibrils such that both the main- and side-chain torsion angles are close to their optimal values. Moreover, the structure of this peptide in the fibrillar form has a degree of long-range order that is generally associated only with crystalline materials. These findings provide an explanation of the unusual stability and characteristic properties of this form of polypeptide assembly.
NASA Astrophysics Data System (ADS)
Powell, C. J.; Werner, W. S. M.; Smekal, W.
2007-09-01
We report on the use of the NIST Database for the Simulation of Electron Spectra for Surface Analysis (SESSA) to determine N 1s, O 1s, and Si 2p3/2 photoelectron intensities for a 25 Å SiON film on a Si substrate with different distributions of N in the film. These simulations were made to assess the distinguishability of angle-resolved x-ray photoelectron spectroscopy (ARXPS) signals for each N distribution. Our approach differs from conventional simulations of ARXPS data in that we do not neglect elastic scattering of the photoelectrons and the finite solid angle of the analyzer. Appreciable dispersion of the photoelectron intensities was found only for the N 1s intensities at an emission angle of 75° (with respect to the surface normal). Conventional analyses of ARXPS data that include such large emission angles are unlikely to be valid due to angle-dependent changes of the attenuation length. We demonstrate the magnitude of elastic-scattering and analyzer solid-angle effects on the calculated angular distributions.
Three-dimensional superconducting gap in FeSe from angle-resolved photoemission spectroscopy
NASA Astrophysics Data System (ADS)
Kushnirenko, Y. S.; Fedorov, A. V.; Haubold, E.; Thirupathaiah, S.; Wolf, T.; Aswartham, S.; Morozov, I.; Kim, T. K.; Büchner, B.; Borisenko, S. V.
2018-05-01
We present a systematic angle-resolved photoemission spectroscopy study of the superconducting gap in FeSe. The gap function is determined in a full Brillouin zone including all Fermi surfaces and kz dependence. We find significant anisotropy of the superconducting gap in all momentum directions. While the in-plane anisotropy can be explained by both nematicity-induced pairing anisotropy and orbital-selective pairing, the kz anisotropy requires an additional refinement of the theoretical approaches.
Method of orthogonally splitting imaging pose measurement
NASA Astrophysics Data System (ADS)
Zhao, Na; Sun, Changku; Wang, Peng; Yang, Qian; Liu, Xintong
2018-01-01
In order to meet the aviation's and machinery manufacturing's pose measurement need of high precision, fast speed and wide measurement range, and to resolve the contradiction between measurement range and resolution of vision sensor, this paper proposes an orthogonally splitting imaging pose measurement method. This paper designs and realizes an orthogonally splitting imaging vision sensor and establishes a pose measurement system. The vision sensor consists of one imaging lens, a beam splitter prism, cylindrical lenses and dual linear CCD. Dual linear CCD respectively acquire one dimensional image coordinate data of the target point, and two data can restore the two dimensional image coordinates of the target point. According to the characteristics of imaging system, this paper establishes the nonlinear distortion model to correct distortion. Based on cross ratio invariability, polynomial equation is established and solved by the least square fitting method. After completing distortion correction, this paper establishes the measurement mathematical model of vision sensor, and determines intrinsic parameters to calibrate. An array of feature points for calibration is built by placing a planar target in any different positions for a few times. An terative optimization method is presented to solve the parameters of model. The experimental results show that the field angle is 52 °, the focus distance is 27.40 mm, image resolution is 5185×5117 pixels, displacement measurement error is less than 0.1mm, and rotation angle measurement error is less than 0.15°. The method of orthogonally splitting imaging pose measurement can satisfy the pose measurement requirement of high precision, fast speed and wide measurement range.
Electron beam imaging and spectroscopy of plasmonic nanoantenna resonances
NASA Astrophysics Data System (ADS)
Vesseur, E. J. R.
2011-07-01
Nanoantennas are metal structures that provide strong optical coupling between a nanoscale volume and the far field. This coupling is mediated by surface plasmons, oscillations of the free electrons in the metal. Increasing the control over the resonant plasmonic field distribution opens up a wide range of applications of nanoantennas operating both in receiving and transmitting mode. This thesis presents how the dispersion and confinement of surface plasmons in nanoantennas are resolved and further engineered. Fabrication of nanostructures is done using focused ion beam milling (FIB) in metallic surfaces. We demonstrate that patterning in single-crystal substrates allows us to precisely control the geometry in which plasmons are confined. The nanoscale properties of the resonant plasmonic fields are resolved using a new technique developed in this thesis: angle- and polarization controlled cathodoluminescence (CL) imaging spectroscopy. The use of a tightly focused electron beam allows us to probe the optical antenna properties with deep subwavelength resolution. We show using this technique that nanoantennas consisting of 500-1200 nm long polycrystalline Au nanowires support standing plasmon waves. We directly observe the plasmon wavelengths which we use to derive the dispersion relation of guided nanowire plasmons. A 590-nm-long ridge-shaped nanoantenna was fabricated using FIB milling on a single-crystal Au substrate, demonstrating a level of control over the fabrication impossible with polycrystalline metals. CL experiments show that the ridge supports multiple-order resonances. The confinement of surface plasmons to the ridge is confirmed by boundary-element-method (BEM) calculations. The resonant modes in plasmonic whispering gallery cavities consisting of a FIB-fabricated circular groove are resolved. We find an excellent agreement between boundary element method calculations and the measured CL emission from the ring-shaped cavities. The calculations show that the ring supports resonances with increasing azimuthal or radial order. The smallest cavity fits only one wavelength in its circumference. We theoretically show that in these cavities, spontaneous emission can be enhanced over a broad spectral band due to the small modal volume of the plasmon resonances. A Purcell factor >2000 was found. We further study the mode symmetries and coupling of the ring resonances using far-field excitation, fluorescence, angle-resolved cathodoluminescence and photoelectron emission microscopy. We demonstrate spectral reshaping of emitters, mode-specific angular emission patterns, and a mode-selective excitation by incoming light, and we directly resolve the modal fields at high resolution. In the next chapter, we present metal-insulator-metal plasmon waveguides in which we engineer the dispersion to reach a refractive index of zero. Using spatially- and angle-resolved CL we directly observe the spatial mode profiles and determine the dispersion relation of plasmon modes. At the cutoff frequency, the emission pattern corresponds to that of a line dipole antenna demonstrating the entire waveguide is in phase (n=0). A strongly enhanced density of optical states is directly observed at cutoff from the enhanced CL intensity. Finally, we present 5 possible applications: a localized surface plasmon sensor, a plasmon ring laser, template stripping technique, an in-situ monitor of ionoluminescence and cathodoluminescence in a FIB system and a single-photon source.
NASA Astrophysics Data System (ADS)
Nielsen, S. K.; Bindslev, H.; Salewski, M.; Bürger, A.; Delabie, E.; Furtula, V.; Kantor, M.; Korsholm, S. B.; Leipold, F.; Meo, F.; Michelsen, P. K.; Moseev, D.; Oosterbeek, J. W.; Stejner, M.; Westerhof, E.; Woskov, P.; TEXTOR Team
2010-09-01
Here we present collective Thomson scattering measurements of 1D fast-ion velocity distribution functions in neutral beam heated TEXTOR plasmas with sawtooth oscillations. Up to 50% of the fast ions in the centre are redistributed as a consequence of a sawtooth crash. We resolve various directions to the magnetic field. The fast-ion distribution is found to be anisotropic as expected. For a resolved angle of 39° to the magnetic field we find a drop in the fast-ion distribution of 20-40%. For a resolved angle of 83° to the magnetic field the drop is no larger than 20%.
Determination Hypocentre and Focal Mechanism Earthquake of Oct 31, 2016 in Bone, South Sulawesi
NASA Astrophysics Data System (ADS)
Altin Massinai, Muhammad; Fawzy Ismullah M, Muhammad
2018-03-01
Indonesian Meteorology, Climatology and Geophysics Agency (BMKG) recorded an earthquake with M4.6 on at October 31, 2016 at Bone District, around 80 Km northeast form Makassar, South Sulawesi. The earthquake occurred 18:18:14 local time in 4.7°S, 120°E with depth 10 Km. Seismicity around location predicted caused by activity Walennae fault. We reprocessed earthquake data to determine precise hypocentre location and focal mechanism. The P- and S-wave arrival time got from BMKG used as input HYPOELLIPSE code to determine hypocentre. The results showed that the earthquake occurred 10:18:14.46 UTC in 4.638°S, 119.966°E with depth 24.76 Km. The hypocentre resolved 10 Km fix depth and had lower travel time residual than BMKG result. Focal mechanism determination used Azmtak code based on the first arrival polarity at earthquake waveform manually picked. The result showed a reverse mechanism with strike direction 38°, dip 44°, rake angle 134° on fault plane I and strike direction 164°, dip 60°, rake angle 56° on fault plane II. So, the earthquake which may be related to a reverse East Walennae Fault.
NASA Astrophysics Data System (ADS)
Anzai, Hiroaki; Takakura, Ryosuke; Ono, Yusuke; Ishihara, Suzuna; Sato, Hitoshi; Namatame, Hirofumi; Taniguchi, Masaki; Matsui, Toshiyuki; Noguchi, Satoru; Hosokoshi, Yuko
2018-05-01
We study the electronic structure of p-trifluoromethylphenyl nitronyl nitroxide (p-CF3PNN), which forms a one-dimensional alternating antiferromagnetic chain of molecules, using angle-resolved photoemission spectroscopy. A singly occupied molecular orbital (SOMO) is observed clearly at ∼ 2 eV in the valence-band spectra. The small band gap and the overlap between the SOMO orbitals in the NO groups are associated with the antiferromagnetic interaction between neighboring spins.
Yamamoto, Yo-ichi; Suzuki, Yoshi-Ichi; Tomasello, Gaia; Horio, Takuya; Karashima, Shutaro; Mitríc, Roland; Suzuki, Toshinori
2014-05-09
We present time- and angle-resolved photoemission spectroscopy of trapped electrons near liquid surfaces. Photoemission from the ground state of a hydrated electron at 260 nm is found to be isotropic, while anisotropic photoemission is observed for the excited states of 1,4-diazabicyclo[2,2,2]octane and I- in aqueous solutions. Our results indicate that surface and subsurface species create hydrated electrons in the bulk side. No signature of a surface-bound electron has been observed.
Kim, Jong-Ahn; Kim, Jae Wan; Kang, Chu-Shik; Jin, Jonghan; Eom, Tae Bong
2011-11-01
We present an angle generator with high resolution and accuracy, which uses multiple ultrasonic motors and a self-calibratable encoder. A cylindrical air bearing guides a rotational motion, and the ultrasonic motors achieve high resolution over the full circle range with a simple configuration. The self-calibratable encoder can compensate the scale error of a divided circle (signal period: 20") effectively by applying the equal-division-averaged method. The angle generator configures a position feedback control loop using the readout of the encoder. By combining the ac and dc operation mode, the angle generator produced stepwise angular motion with 0.005" resolution. We also evaluated the performance of the angle generator using a precision angle encoder and an autocollimator. The expanded uncertainty (k = 2) in the angle generation was estimated less than 0.03", which included the calibrated scale error and the nonlinearity error. © 2011 American Institute of Physics
Solar axion search technique with correlated signals from multiple detectors
Xu, Wenqin; Elliott, Steven R.
2017-01-25
The coherent Bragg scattering of photons converted from solar axions inside crystals would boost the signal for axion-photon coupling enhancing experimental sensitivity for these hypothetical particles. Knowledge of the scattering angle of solar axions with respect to the crystal lattice is required to make theoretical predications of signal strength. Hence, both the lattice axis angle within a crystal and the absolute angle between the crystal and the Sun must be known. In this paper, we examine how the experimental sensitivity changes with respect to various experimental parameters. We also demonstrate that, in a multiple-crystal setup, knowledge of the relative axismore » orientation between multiple crystals can improve the experimental sensitivity, or equivalently, relax the precision on the absolute solar angle measurement. However, if absolute angles of all crystal axes are measured, we find that a precision of 2°–4° will suffice for an energy resolution of σ E = 0.04E and a flat background. Lastly, we also show that, given a minimum number of detectors, a signal model averaged over angles can substitute for precise crystal angular measurements, with some loss of sensitivity.« less
High-performance time-resolved fluorescence by direct waveform recording.
Muretta, Joseph M; Kyrychenko, Alexander; Ladokhin, Alexey S; Kast, David J; Gillispie, Gregory D; Thomas, David D
2010-10-01
We describe a high-performance time-resolved fluorescence (HPTRF) spectrometer that dramatically increases the rate at which precise and accurate subnanosecond-resolved fluorescence emission waveforms can be acquired in response to pulsed excitation. The key features of this instrument are an intense (1 μJ/pulse), high-repetition rate (10 kHz), and short (1 ns full width at half maximum) laser excitation source and a transient digitizer (0.125 ns per time point) that records a complete and accurate fluorescence decay curve for every laser pulse. For a typical fluorescent sample containing a few nanomoles of dye, a waveform with a signal/noise of about 100 can be acquired in response to a single laser pulse every 0.1 ms, at least 10(5) times faster than the conventional method of time-correlated single photon counting, with equal accuracy and precision in lifetime determination for lifetimes as short as 100 ps. Using standard single-lifetime samples, the detected signals are extremely reproducible, with waveform precision and linearity to within 1% error for single-pulse experiments. Waveforms acquired in 0.1 s (1000 pulses) with the HPTRF instrument were of sufficient precision to analyze two samples having different lifetimes, resolving minor components with high accuracy with respect to both lifetime and mole fraction. The instrument makes possible a new class of high-throughput time-resolved fluorescence experiments that should be especially powerful for biological applications, including transient kinetics, multidimensional fluorescence, and microplate formats.
Servomotor and Controller Having Large Dynamic Range
NASA Technical Reports Server (NTRS)
Alhorn, Dean C.; Howard, David E.; Smith, Dennis A.; Dutton, Ken; Paulson, M. Scott
2007-01-01
A recently developed micro-commanding rotational-position-control system offers advantages of less mechanical complexity, less susceptibility to mechanical resonances, less power demand, less bulk, less weight, and lower cost, relative to prior rotational-position-control systems based on stepping motors and gear drives. This system includes a digital-signal- processor (DSP)-based electronic controller, plus a shaft-angle resolver and a servomotor mounted on the same shaft. Heretofore, micro-stepping has usually been associated with stepping motors, but in this system, the servomotor is micro-commanded in response to rotational-position feedback from the shaft-angle resolver. The shaft-angle resolver is of a four-speed type chosen because it affords four times the resolution of a single-speed resolver. A key innovative aspect of this system is its position-feedback signal- conditioning circuits, which condition the resolver output signal for multiple ranges of rotational speed. In the preferred version of the system, two rotational- speed ranges are included, but any number of ranges could be added to expand the speed range or increase resolution in particular ranges. In the preferred version, the resolver output is conditioned with two resolver-to-digital converters (RDCs). One RDC is used for speeds from 0.00012 to 2.5 rpm; the other RDC is used for speeds of 2.5 to 6,000 rpm. For the lower speed range, the number of discrete steps of RDC output per revolution was set at 262,144 (4 quadrants at 16 bits per quadrant). For the higher speed range, the number of discrete steps per revolution was set at 4,096 (4 quadrants at 10 bits per quadrant).
Electron-helium S-wave model benchmark calculations. I. Single ionization and single excitation
NASA Astrophysics Data System (ADS)
Bartlett, Philip L.; Stelbovics, Andris T.
2010-02-01
A full four-body implementation of the propagating exterior complex scaling (PECS) method [J. Phys. B 37, L69 (2004)] is developed and applied to the electron-impact of helium in an S-wave model. Time-independent solutions to the Schrödinger equation are found numerically in coordinate space over a wide range of energies and used to evaluate total and differential cross sections for a complete set of three- and four-body processes with benchmark precision. With this model we demonstrate the suitability of the PECS method for the complete solution of the full electron-helium system. Here we detail the theoretical and computational development of the four-body PECS method and present results for three-body channels: single excitation and single ionization. Four-body cross sections are presented in the sequel to this article [Phys. Rev. A 81, 022716 (2010)]. The calculations reveal structure in the total and energy-differential single-ionization cross sections for excited-state targets that is due to interference from autoionization channels and is evident over a wide range of incident electron energies.
NASA Astrophysics Data System (ADS)
Chen, Xin; Wang, Shuhong; Liu, Zhen; Wei, Xizhang
2017-07-01
Localization of a source whose half-wavelength is smaller than the array aperture would suffer from serious phase ambiguity problem, which also appears in recently proposed phase-based algorithms. In this paper, by using the centro-symmetry of fixed uniform circular array (UCA) with even number of sensors, the source's angles and range can be decoupled and a novel ambiguity resolving approach is addressed for phase-based algorithms of source's 3-D localization (azimuth angle, elevation angle, and range). In the proposed method, by using the cosine property of unambiguous phase differences, ambiguity searching and actual-value matching are first employed to obtain actual phase differences and corresponding source's angles. Then, the unambiguous angles are utilized to estimate the source's range based on a one dimension multiple signal classification (1-D MUSIC) estimator. Finally, simulation experiments investigate the influence of step size in search and SNR on performance of ambiguity resolution and demonstrate the satisfactory estimation performance of the proposed method.
Local atomic structure of Fe/Cr multilayers: Depth-resolved method
NASA Astrophysics Data System (ADS)
Babanov, Yu. A.; Ponomarev, D. A.; Devyaterikov, D. I.; Salamatov, Yu. A.; Romashev, L. N.; Ustinov, V. V.; Vasin, V. V.; Ageev, A. L.
2017-10-01
A depth-resolved method for the investigation of the local atomic structure by combining data of X-ray reflectivity and angle-resolved EXAFS is proposed. The solution of the problem can be divided into three stages: 1) determination of the element concentration profile with the depth z from X-ray reflectivity data, 2) determination of the X-ray fluorescence emission spectrum of the element i absorption coefficient μia (z,E) as a function of depth and photon energy E using the angle-resolved EXAFS data Iif (E , ϑl) , 3) determination of partial correlation functions gij (z , r) as a function of depth from μi (z , E) . All stages of the proposed method are demonstrated on a model example of a multilayer nanoheterostructure Cr/Fe/Cr/Al2O3. Three partial pair correlation functions are obtained. A modified Levenberg-Marquardt algorithm and a regularization method are applied.
Angle-resolved reflection spectroscopy of high-quality PMMA opal crystal
NASA Astrophysics Data System (ADS)
Nemtsev, Ivan V.; Tambasov, Igor A.; Ivanenko, Alexander A.; Zyryanov, Victor Ya.
2018-02-01
PMMA opal crystal was prepared by a simple hybrid method, which includes sedimentation, meniscus formation and evaporation. We investigated three surfaces of this crystal by angle-resolved reflective light spectroscopy and SEM study. The angle-resolved reflective measurements were carried out in the 400-1100 nm range. We have determined the high-quality ordered surface of the crystal region. Narrow particle size distribution of the surface has been revealed. The average particle diameter obtained with SEM was nearly 361 nm. The most interesting result was that reflectivity of the surface turned out up to 98% at normal light incidence. Using a fit of dependences of the maximum reflectivity wavelength from an angle based on the Bragg-Snell law, the wavelength of maximum 0° reflectivity, the particle diameter and the fill factor have been determined. For the best surface maximum reflectivity wavelength of a 0° angle was estimated to be 869 nm. The particle diameter and fill factor were calculated as 372 nm and 0.8715, respectively. The diameter obtained by fitting is in excellent agreement with the particle diameter obtained with SEM. The reflectivity maximum is assumed to increase significantly when increasing the fill factor. We believe that using our simple approach to manufacture PMMA opal crystals will significantly increase the fabrication of high-quality photonic crystal templates and thin films.
Scanning system for angle-resolved low-coherence interferometry.
Steelman, Zachary A; Ho, Derek; Chu, Kengyeh K; Wax, Adam
2017-11-15
Angle-resolved low-coherence interferometry (a/LCI) detects precancer by enabling depth-resolved measurements of nuclear morphology in vivo. A significant limitation of a/LCI is the point-probe nature of the method, sampling <0.5 mm 2 before probe relocation is necessary. In this work, we demonstrate a scanning method capable of assessing an area >100 mm 2 without repositioning. By utilizing a reflection-only three-optic rotator prism and a two-axis scanning mirror, we demonstrate radial scans of a sample with a linear range of 12 mm and a full rotational range of 180°. Use of this design will improve the diagnostic utility of a/LCI for wide-area screening of tissue health.
A scanning system for angle-resolved low-coherence interferometry
Steelman, Zachary A.; Ho, Derek; Chu, Kengyeh K.; Wax, Adam
2018-01-01
Angle-resolved low-coherence interferometry (a/LCI) detects precancer by enabling depth-resolved measurements of nuclear morphology in vivo. A significant limitation of a/LCI is the point-probe nature of the method, sampling <0.5 mm2 before probe relocation is necessary. In this work, we demonstrate a scanning method capable of assessing an area >100 mm2 without repositioning. By utilizing a reflection-only three-optic rotator (ROTOR) prism and two-axis scanning mirror, we demonstrate radial scans of a sample with a linear range of 12 mm and a full rotational range of 180°. Use of this design will improve the diagnostic utility of a/LCI for wide-area screening of tissue health. PMID:29140317
DOE Office of Scientific and Technical Information (OSTI.GOV)
Falcinelli, Stefano, E-mail: stefano.falcinelli@unipg.it; Vecchiocattivi, Franco; Bartocci, Alessio
2015-10-28
A combined analysis of both new (energy spectra of emitted electrons) and previously published (ionization cross sections) experimental data, measured under the same conditions and concerning electronically excited lighter noble gas –NH{sub 3} collisional autoionization processes, is carried out. Such an analysis, performed by exploiting a formulation of the full potential energy surface both in the real and imaginary parts, provides direct information on energetics, structure, and lifetime of the intermediate collision complex over all the configuration space. The marked anisotropy in the attraction of the real part, driving the approach of reagents, and the selective role of the imaginarymore » component, associated to the charge transfer coupling between entrance and exit channels, suggests that reactive events occur almost exclusively in the molecular hemisphere containing the nitrogen lone pair. Crucial details on the stereo-dynamics of elementary collisional autoionization processes are then obtained, in which the open shell nature of the disclosed ionic core of metastable atom plays a crucial role. The same analysis also suggests that the strength of the attraction and the anisotropy of the interaction increases regularly along the series Ne{sup *}({sup 3}P), He{sup *}({sup 3}S), He{sup *}({sup 1}S)–NH{sub 3}. These findings can be ascribed to the strong rise of the metastable atom electronic polarizability (deformability) along the series. The obtained results can stimulate state of the art ab initio calculations focused on specific features of the transition state (energetics, structure, lifetime, etc.) which can be crucial for a further improvement of the adopted treatment and to better understand the nature of the leading interaction components which are the same responsible for the formation of the intermolecular halogen and hydrogen bond.« less
A new fitting method for measurement of the curvature radius of a short arc with high precision
NASA Astrophysics Data System (ADS)
Tao, Wei; Zhong, Hong; Chen, Xiao; Selami, Yassine; Zhao, Hui
2018-07-01
The measurement of an object with a short arc is widely encountered in scientific research and industrial production. As the most classic method of arc fitting, the least squares fitting method suffers from low precision when it is used for measurement of arcs with smaller central angles and fewer sampling points. The shorter the arc, the lower is the measurement accuracy. In order to improve the measurement precision of short arcs, a parameter constrained fitting method based on a four-parameter circle equation is proposed in this paper. The generalized Lagrange function was introduced together with the optimization by gradient descent method to reduce the influence from noise. The simulation and experimental results showed that the proposed method has high precision even when the central angle drops below 4° and it has good robustness when the noise standard deviation rises to 0.4 mm. This new fitting method is suitable for the high precision measurement of short arcs with smaller central angles without any prior information.
NASA Astrophysics Data System (ADS)
Ueda, Yoshihiro; Suzuki, Yasumitsu; Watanabe, Kazuyuki
2018-02-01
Angle-resolved secondary electron emission (ARSEE) spectra were analyzed for two-dimensional atomic sheets using a time-dependent first-principles simulation of electron scattering. We demonstrate that the calculated ARSEE spectra capture the unoccupied band structure of the atomic sheets. The excitation dynamics that lead to SEE have also been revealed by the time-dependent Kohn-Sham decomposition scheme. In the present study, the mechanism for the experimentally observed ARSEE from atomic sheets is elucidated with respect to both energetics and the dynamical aspects of SEE.
Tadich, A; Riley, J; Thomsen, L; Cowie, B C C; Gladys, M J
2011-10-21
Chiral interfaces and substrates are of increasing importance in the field of enantioselective chemistry. To fully understand the enantiospecific interactions between chiral adsorbate molecules and the chiral substrate, it is vital that the chiral orientation of the substrate is known. In this Letter we demonstrate that full-hemisphere angle-resolved photoemission permits straightforward identification of the orientation of a chiral surface. The technique can be applied to any solid state system for which photoemission measurements are possible. © 2011 American Physical Society
Dissociative recombination of HCl+
NASA Astrophysics Data System (ADS)
Larson, Åsa; Fonseca dos Santos, Samantha; E. Orel, Ann
2017-08-01
The dissociative recombination of HCl+, including both the direct and indirect mechanisms, is studied. For the direct process, the relevant electronic states are calculated ab initio by combining electron scattering calculations to obtain resonance positions and autoionization widths with multi-reference configuration interaction calculations of the ion and Rydberg states. The cross section for the direct dissociation along electronic resonant states is computed by solution of the time-dependent Schrödinger equation. For the indirect process, an upper bound value for the cross section is obtained using a vibrational frame transformation of the elements of the scattering matrix at energies just above the ionization threshold. Vibrational excitations of the ionic core from the ground vibrational state, v = 0 , to the first three excited vibrational states, v = 1 , v = 2 , and v = 3 , are considered. Autoionization is neglected and the effect of the spin-orbit splitting of the ionic potential energy upon the indirect dissociative recombination cross section is considered. The calculated cross sections are compared to measurements.
Total photoionization cross sections of atomic oxygen from threshold to 44.3A
NASA Technical Reports Server (NTRS)
Angel, G. C.; Samson, James A. R.
1987-01-01
The relative cross section of atomic oxygen for the production of singly charged ions has been remeasured in more detail and extended to cover the wavelength range 44.3 to 910.5 A by the use of synchrotron radiation. In addition, the contribution of multiple ionization to the cross sections has been measured allowing total photoionization cross sections to be obtained below 250 A. The results have been made absolute by normalization to previously measured data. The use of synchrotron radiation has enabled measurements of the continuum cross section to be made between the numerous autoionizing resonances that occur near the ionization thresholds. This in turn has allowed a more critical comparison of the various theoretical estimates of the cross section to be made. The series of autoionizing resonances leading to the 4-P state of the oxygen ion have been observed for the first time in an ionization type experiment and their positions compared with both theory and previous photographic recordings.
Dissociative recombination of HCl.
Larson, Åsa; Fonseca Dos Santos, Samantha; E Orel, Ann
2017-08-28
The dissociative recombination of HCl + , including both the direct and indirect mechanisms, is studied. For the direct process, the relevant electronic states are calculated ab initio by combining electron scattering calculations to obtain resonance positions and autoionization widths with multi-reference configuration interaction calculations of the ion and Rydberg states. The cross section for the direct dissociation along electronic resonant states is computed by solution of the time-dependent Schrödinger equation. For the indirect process, an upper bound value for the cross section is obtained using a vibrational frame transformation of the elements of the scattering matrix at energies just above the ionization threshold. Vibrational excitations of the ionic core from the ground vibrational state, v = 0, to the first three excited vibrational states, v = 1, v = 2, and v = 3, are considered. Autoionization is neglected and the effect of the spin-orbit splitting of the ionic potential energy upon the indirect dissociative recombination cross section is considered. The calculated cross sections are compared to measurements.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Saquet, N.; Holland, D. M. P.; Pratt, S. T.
We present photoelectron energy and angular distributions for resonant two-photon ionization via several low-lying Rydberg states of atomic Kr. The experiments were performed by using synchrotron radiation to pump the Rydberg states and a continuous-wave laser to probe them. Photoelectron images, recorded with both linear and circular polarized pump and probe light, were obtained in coincidence with mass-analyzed Kr ions. The photoelectron angular distributions and branching ratios for direct ionization into the Kr+ P-2(3/2) and P-2(1/2) spin-orbit continua show considerable dependence on the intermediate level, as well as on the polarizations of the pump and probe light. Photoelectron images weremore » also recorded with several polarization combinations following two-color excitation of the (P-2(1/2))5f[5/2](2) autoionizing resonance. These results are compared with the results of recent work on the corresponding autoionizing resonance in atomic Xe [E. V. Gryzlova et al., New J. Phys. 17, 043054 (2015)].« less
Hoesch, M; Kim, T K; Dudin, P; Wang, H; Scott, S; Harris, P; Patel, S; Matthews, M; Hawkins, D; Alcock, S G; Richter, T; Mudd, J J; Basham, M; Pratt, L; Leicester, P; Longhi, E C; Tamai, A; Baumberger, F
2017-01-01
A synchrotron radiation beamline in the photon energy range of 18-240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation undulator, a high resolution monochromator, a re-focussing system to form a beam spot of 50 × 50 μm 2 , and an end station for angle-resolved photoelectron spectroscopy (ARPES) including a 6-degrees-of-freedom cryogenic sample manipulator. The beamline design and its performance allow for a highly productive and precise use of the ARPES technique at an energy resolution of 10-15 meV for fast k-space mapping studies with a photon flux up to 2 ⋅ 10 13 ph/s and well below 3 meV for high resolution spectra.
Dynamic tailoring of surface plasmon polaritons through incident angle modulation.
Qiu, Peizhen; Zhang, Dawei; Jing, Ming; Lu, Taiguo; Yu, Binbin; Zhan, Qiwen; Zhuang, Songlin
2018-04-16
Dynamic tailoring of the propagating surface plasmon polaritons (SPPs) through incident angle modulation is proposed and numerically demonstrated. The generation and tailoring mechanism of the SPPs are discussed. The relationship formula between the incident angle and the generated SPP wave vector direction is theoretically derived. The correctness of the formula is verified with three different approaches using finite difference time domain method. Using this formula, the generated SPP wave vector direction can be precisely modulated by changing the incident angle. The precise modulation results of two dimensional Bessel-like SPP beam and SPP bottle beam array are given. The results can deepen the understanding of the generation and modulation mechanism of the SPPs.
NASA Astrophysics Data System (ADS)
Gu, Ming Feng
2018-02-01
FAC calculates various atomic radiative and collisional processes, including radiative transition rates, collisional excitation and ionization by electron impact, energy levels, photoionization, and autoionization, and their inverse processes radiative recombination and dielectronic capture. The package also includes a collisional radiative model to construct synthetic spectra for plasmas under different physical conditions.
Safronova, U. I.; Safronova, A. S.; Beiersdorfer, P.
2016-11-02
Energy levels, radiative transition probabilities, and autoionization rates for [Ni]more » $$4{s}^{2}4{p}^{6}{nl}$$, [Ni]$$4{s}^{2}4{p}^{5}4l^{\\prime} {nl}$$ ($$l^{\\prime} =d,f,n$$ = 4–7), [Ni]$$4s4{p}^{6}4l^{\\prime} {nl}$$, ($$l^{\\prime} =d,f,n$$ = 4–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} {nl}$$ (n = 5–7), and [Ni]$$4s4{p}^{6}6l^{\\prime} {nl}$$ (n = 6–7) states in Rb-like tungsten (W37+) are calculated using the relativistic many-body perturbation theory method (RMBPT code) and the Hartree–Fock-relativistic method (COWAN code). Autoionizing levels above the [Ni]$$4{s}^{2}4{p}^{6}$$ threshold are considered. It is found that configuration mixing among [Ni]$$4{s}^{2}4{p}^{5}4l^{\\prime} {nl}$$ and [Ni]$$4s4{p}^{6}4l^{\\prime} {nl}$$ plays an important role for all atomic characteristics. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and dielectronic recombination (DR) rate coefficients are determined for the [Ni]$$4{s}^{2}4{p}^{6}{nl}$$ (n = 4–7) singly excited states, as well as the [Ni]$$4{s}^{2}4{p}^{5}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{5}4{fnl}$$, [Ni]$$4s4{p}^{6}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{6}4{fnl}$$, (n = 4–6), and [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} 5l$$ doubly excited nonautoionizing states in Rb-like W37+ ion. Contributions from the [Ni]$$4s24{p}^{6}4{fnl}$$ (n = 6–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} {nl}$$ (n = 5–6), and [Ni]$$4{s}^{2}4{p}^{5}6l^{\\prime} {nl}$$ (n = 6–7) doubly excited autoionizing states are evaluated numerically. The high-n state (with n up to 500) contributions are very important for high temperatures. These contributions are determined by using a scaling procedure. Synthetic dielectronic satellite spectra from Rb-like W are simulated in a broad spectral range from 8 to 70 Å. Here, these calculations provide highly accurate values for a number of W 37+ properties useful for a variety of applications including for fusion applications.« less
Precision and repeatability of the Optotrak 3020 motion measurement system.
States, R A; Pappas, E
2006-01-01
Several motion analysis systems are used by researchers to quantify human motion and to perform accurate surgical procedures. The Optotrak 3020 is one of these systems and despite its widespread use there is not any published information on its precision and repeatability. We used a repeated measures design study to evaluate the precision and repeatability of the Optotrak 3020 by measuring distance and angle in three sessions, four distances and three conditions (motion, static vertical, and static tilted). Precision and repeatability were found to be excellent for both angle and distance although they decreased with increasing distance from the sensors and with tilt from the plane of the sensors. Motion did not have a significant effect on the precision of the measurements. In conclusion, the measurement error of the Optotrak is minimal. Further studies are needed to evaluate its precision and repeatability under human motion conditions.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Kimura, Shin-Ichi; Ito, Takahiro; Hosaka, Masahito
A novel variably polarized angle-resolved photoemission spectroscopy beamline in the vacuum-ultraviolet (VUV) region has been installed at the UVSOR-II 750 MeV synchrotron light source. The beamline is equipped with a 3 m long APPLE-II type undulator with horizontally/vertically linear and right/left circular polarizations, a 10 m Wadsworth type monochromator covering a photon energy range of 6-43 eV, and a 200 mm radius hemispherical photoelectron analyzer with an electron lens of a {+-}18 deg. acceptance angle. Due to the low emittance of the UVSOR-II storage ring, the light source is regarded as an entrance slit, and the undulator light is directlymore » led to a grating by two plane mirrors in the monochromator while maintaining a balance between high-energy resolution and high photon flux. The energy resolving power (h{nu}/{Delta}h{nu}) and photon flux of the monochromator are typically 1x10{sup 4} and 10{sup 12} photons/s, respectively, with a 100 {mu}m exit slit. The beamline is used for angle-resolved photoemission spectroscopy with an energy resolution of a few meV covering the UV-to-VUV energy range.« less
Klein, Thomas; André, Raphael; Wieser, Wolfgang; Pfeiffer, Tom; Huber, Robert
2013-01-01
Joint-aperture optical coherence tomography (JA-OCT) is an angle-resolved OCT method, in which illumination from an active channel is simultaneously probed by several passive channels. JA-OCT increases the collection efficiency and effective sensitivity of the OCT system without increasing the power on the sample. Additionally, JA-OCT provides angular scattering information about the sample in a single acquisition, so the OCT imaging speed is not reduced. Thus, JA-OCT is especially suitable for ultra high speed in-vivo imaging. JA-OCT is compared to other angle-resolved techniques, and the relation between joint aperture imaging, adaptive optics, coherent and incoherent compounding is discussed. We present angle-resolved imaging of the human retina at an axial scan rate of 1.68 MHz, and demonstrate the benefits of JA-OCT: Speckle reduction, signal increase and suppression of specular and parasitic reflections. Moreover, in the future JA-OCT may allow for the reconstruction of the full Doppler vector and tissue discrimination by analysis of the angular scattering dependence. PMID:23577296
NASA Astrophysics Data System (ADS)
Schmitt, W.; Hormes, J.; Kuetgens, U.; Gries, W. H.
1992-01-01
An apparatus for angle-resolved, wavelength-dispersive x-ray fluorescence spectroscopy with synchrotron radiation has been built and tested at the beam line BN2 of the Bonn electron stretcher and accelerator (ELSA). The apparatus is to be used for nondestructive depth profile analysis of ion-implanted semiconductors as part of the multinational Versailles Project of Advanced Materials and Standards (VAMAS) project on ion-implanted reference materials. In particular, the centroid depths of depth profiles of various implants is to be determined by use of the angle-resolved signal ratio technique. First results of measurements on implants of phosphorus (100 keV, 1016 cm-2) and sulfur (200 keV, 1014 cm-2) in silicon wafers using ``white'' synchrotron radiation are presented and suggest that it should be generally possible to measure the centroid depth of an implant at dose densities as low as 1014 cm-2. Some of the apparative and technical requirements are discussed which are peculiar to the use of synchrotron radiation in general and to the use of nonmonochromatized radiation in particular.
Camber Angle Inspection for Vehicle Wheel Alignments
Young, Jieh-Shian; Hsu, Hong-Yi; Chuang, Chih-Yuan
2017-01-01
This paper introduces an alternative approach to the camber angle measurement for vehicle wheel alignment. Instead of current commercial approaches that apply computation vision techniques, this study aims at realizing a micro-control-unit (MCU)-based camber inspection system with a 3-axis accelerometer. We analyze the precision of the inspection system for the axis misalignments of the accelerometer. The results show that the axes of the accelerometer can be aligned to the axes of the camber inspection system imperfectly. The calibrations that can amend these axis misalignments between the camber inspection system and the accelerometer are also originally proposed since misalignments will usually happen in fabrications of the inspection systems. During camber angle measurements, the x-axis or z-axis of the camber inspection system and the wheel need not be perfectly aligned in the proposed approach. We accomplished two typical authentic camber angle measurements. The results show that the proposed approach is applicable with a precision of ±0.015∘ and therefore facilitates the camber measurement process without downgrading the precision by employing an appropriate 3-axis accelerometer. In addition, the measured results of camber angles can be transmitted via the medium such as RS232, Bluetooth, and Wi-Fi. PMID:28165365
Synchronizing Photography For High-Speed-Engine Research
NASA Technical Reports Server (NTRS)
Chun, K. S.
1989-01-01
Light flashes when shaft reaches predetermined angle. Synchronization system facilitates visualization of flow in high-speed internal-combustion engines. Designed for cinematography and holographic interferometry, system synchronizes camera and light source with predetermined rotational angle of engine shaft. 10-bit resolution of absolute optical shaft encoder adapted, and 2 to tenth power combinations of 10-bit binary data computed to corresponding angle values. Pre-computed angle values programmed into EPROM's (erasable programmable read-only memories) to use as angle lookup table. Resolves shaft angle to within 0.35 degree at rotational speeds up to 73,240 revolutions per minute.
Precision controllability of the YF-17 airplane
NASA Technical Reports Server (NTRS)
Sisk, T. R.; Mataeny, N. W.
1980-01-01
A flying qualities evaluation conducted on the YF-17 airplane permitted assessment of its precision controllability in the transonic flight regime over the allowable angle of attack range. The precision controllability (tailchase tracking) study was conducted in constant-g and windup turn tracking maneuvers with the command augmentation system (CAS) on, automatic maneuver flaps, and the caged pipper gunsight depressed 70 mils. This study showed that the YF-17 airplane tracks essentially as well at 7 g's to 8 g's as earlier fighters did at 4 g's to 5 g's before they encountered wing rock. The pilots considered the YF-17 airplane one of the best tracking airplanes they had flown. Wing rock at the higher angles of attack degraded tracking precision, and lack of control harmony made precision controllability more difficult. The revised automatic maneuver flap schedule incorporated in the airplane at the time of the tests did not appear to be optimum. The largest tracking errors and greatest pilot workload occurred at high normal load factors at low angles of attack. The pilots reported that the high-g maneuvers caused some tunnel vision and that they found it difficult to think clearly after repeated maneuvers.
Temperature-induced band shift in bulk γ-InSe by angle-resolved photoemission spectroscopy
NASA Astrophysics Data System (ADS)
Xu, Huanfeng; Wang, Wei; Zhao, Yafei; Zhang, Xiaoqian; Feng, Yue; Tu, Jian; Gu, Chenyi; Sun, Yizhe; Liu, Chang; Nie, Yuefeng; Edmond Turcu, Ion C.; Xu, Yongbing; He, Liang
2018-05-01
Indium selenide (InSe) has recently become popular research topics because of its unique layered crystal structure, direct band gap and high electron mobilities. In this work, we have acquired the electronic structure of bulk γ-InSe at various temperatures using angle-resolved photoemission spectroscopy (ARPES). We have also found that as the temperature decreases, the valence bands of γ-InSe exhibit a monotonic shift to lower binding energies. This band shift is attributed to the change of lattice parameters and has been validated by variable temperature X-ray diffraction measurements and theoretical calculations.
NASA Astrophysics Data System (ADS)
Schmitt, W.; Drotbohm, P.; Rothe, J.; Hormes, J.; Ottermann, C. R.; Bange, K.
1995-05-01
Thickness measurements by the method of angle-resolved, self-ratio X-ray fluorescence spectrometry (AR/SR/XFS) have been carried out on thin solid films using monochromatized synchrotron radiation at the Bonn storage ring ELSA. Synchrotron radiation was monochromatized by means of a double-crystal monochromator and fluorescence radiation was detected by a Si(Li) semiconductor detector. The results for sample systems consisting of Au on Si, Cr on SiO2 and TiO2 on alkali-free glass are very satisfactory and agree well with results obtained by other methods.
Angle-Resolved Second-Harmonic Light Scattering from Colloidal Particles
DOE Office of Scientific and Technical Information (OSTI.GOV)
Yang, N.; Angerer, W. E.; Yodh, A. G.
2001-09-03
We report angle-resolved second-harmonic generation (SHG) measurements from suspensions of centrosymmetric micron-size polystyrene spheres with surface-adsorbed dye (malachite green). The second-harmonic scattering profiles differ qualitatively from linear light scattering profiles of the same particles. We investigated these radiation patterns using several polarization configurations and particle diameters. We introduce a simple Rayleigh-Gans-Debye model to account for the SHG scattering anisotropy. The model compares favorably with our experimental data. Our measurements suggest scattering anisotropy may be used to isolate particle nonlinear optics from other bulk nonlinear optical effects in suspension.
Angle-Resolved Photoemission of Solvated Electrons in Sodium-Doped Clusters.
West, Adam H C; Yoder, Bruce L; Luckhaus, David; Saak, Clara-Magdalena; Doppelbauer, Maximilian; Signorell, Ruth
2015-04-16
Angle-resolved photoelectron spectroscopy of the unpaired electron in sodium-doped water, methanol, ammonia, and dimethyl ether clusters is presented. The experimental observations and the complementary calculations are consistent with surface electrons for the cluster size range studied. Evidence against internally solvated electrons is provided by the photoelectron angular distribution. The trends in the ionization energies seem to be mainly determined by the degree of hydrogen bonding in the solvent and the solvation of the ion core. The onset ionization energies of water and methanol clusters do not level off at small cluster sizes but decrease slightly with increasing cluster size.
Gauquelin, N; van den Bos, K H W; Béché, A; Krause, F F; Lobato, I; Lazar, S; Rosenauer, A; Van Aert, S; Verbeeck, J
2017-10-01
Nowadays, aberration corrected transmission electron microscopy (TEM) is a popular method to characterise nanomaterials at the atomic scale. Here, atomically resolved images of nanomaterials are acquired, where the contrast depends on the illumination, imaging and detector conditions of the microscope. Visualization of light elements is possible when using low angle annular dark field (LAADF) STEM, annular bright field (ABF) STEM, integrated differential phase contrast (iDPC) STEM, negative spherical aberration imaging (NCSI) and imaging STEM (ISTEM). In this work, images of a NdGaO 3 -La 0.67 Sr 0.33 MnO 3 (NGO-LSMO) interface are quantitatively evaluated by using statistical parameter estimation theory. For imaging light elements, all techniques are providing reliable results, while the techniques based on interference contrast, NCSI and ISTEM, are less robust in terms of accuracy for extracting heavy column locations. In term of precision, sample drift and scan distortions mainly limits the STEM based techniques as compared to NCSI. Post processing techniques can, however, partially compensate for this. In order to provide an outlook to the future, simulated images of NGO, in which the unavoidable presence of Poisson noise is taken into account, are used to determine the ultimate precision. In this future counting noise limited scenario, NCSI and ISTEM imaging will provide more precise values as compared to the other techniques, which can be related to the mechanisms behind the image recording. Copyright © 2017 Elsevier B.V. All rights reserved.
NASA Astrophysics Data System (ADS)
Miller, Patrick J.; Tyack, Peter L.
Investigations of communication systems benefit from concurrent observation of vocal and visible behaviors of individual animals. A device has been developed to identify individual vocalizing resident killer whales ( Orcinus orca) during focal behavioral observations. The device consists of a 2-m, 15-element hydrophone array, which is easily towed behind a small vessel, on-board multi-channel recorders, and real-time signal processing equipment. Acoustic data from the hydrophones are digitized and processed using broadband frequency-domain beamforming to yield frequency-azimuth (FRAZ) and "directo-gram" displays of arriving sounds. Based upon statistical analysis of independent portions of typical killer whale calls, the precision of the angle-of-arrival estimate ranges from ±0° to ±2.5° with a mean precision of ±1.5°. Echolocation clicks also are resolved precisely with a typical -6 dB mainlobe width of ±2.0°. Careful positioning of the array relative to the animals minimizes the effects of depth ambiguities and allows identification of individual sources in many circumstances. Several strategies for identifying vocalizing individuals are discussed and an example of a successful identification is described. Use of the array with resident killer whales did not interfere with vessel maneuverability, animal tracking, or behavioral sampling of focal individuals. This localization technique has promise for advancing the abilities of researchers to conduct unbiased behavioral and acoustic sampling of individual free-ranging cetaceans.
NASA Astrophysics Data System (ADS)
Robert, Clélia; Conan, Jean-Marc; Wolf, Peter
2016-06-01
Bidirectional ground-satellite laser links suffer from turbulence-induced scintillation and phase distortion. We study how turbulence impacts on coherent detection capacity and on the associated phase noise that restricts clock transfer precision. We evaluate the capacity to obtain a two-way cancellation of atmospheric effects despite the asymmetry between up and down link that limits the link reciprocity. For ground-satellite links, the asymmetry is induced by point-ahead angle and possibly the use, for the ground terminal, of different transceiver diameters, in reception and emission. The quantitative analysis is obtained thanks to refined end- to-end simulations under realistic turbulence and wind conditions as well as satellite cinematic. These temporally resolved simulations allow characterizing the coherent detection in terms of time series of heterodyne efficiency for different system parameters. We show that Tip/Tilt correction on ground is mandatory at reception for the down link and as a pre-compensation of the up link. Good correlation between up and down phase noise is obtained even with asymmetric apertures of the ground transceiver and in spite of pointing ahead angle. The reduction to less than 1 rad2 of the two-way differential phase noise is very promising for clock comparisons.
NASA Technical Reports Server (NTRS)
Predina, Joseph P. (Inventor)
1989-01-01
A digital-to-synchro converter is provided where a binary input code specifies a desired shaft angle and where an resolver type position transducer is employed with additional circuitry to generate a shaft position error signal indicative of the angular difference between the desired shaft angle and the actual shaft angle. The additional circuitry corrects for known and calculated errors in the shaft position detection process and equipment.
Federal Register 2010, 2011, 2012, 2013, 2014
2010-07-07
... the stator and the rotor parts of the AoA [angle of attack] vane position resolvers. This oil residue... extent, it could lead to a late activation of the angle of attack protection, which in combination with light at high angle of attack would constitute an unsafe condition. The proposed AD would require...
The Use of Scale-Dependent Precision to Increase Forecast Accuracy in Earth System Modelling
NASA Astrophysics Data System (ADS)
Thornes, Tobias; Duben, Peter; Palmer, Tim
2016-04-01
At the current pace of development, it may be decades before the 'exa-scale' computers needed to resolve individual convective clouds in weather and climate models become available to forecasters, and such machines will incur very high power demands. But the resolution could be improved today by switching to more efficient, 'inexact' hardware with which variables can be represented in 'reduced precision'. Currently, all numbers in our models are represented as double-precision floating points - each requiring 64 bits of memory - to minimise rounding errors, regardless of spatial scale. Yet observational and modelling constraints mean that values of atmospheric variables are inevitably known less precisely on smaller scales, suggesting that this may be a waste of computer resources. More accurate forecasts might therefore be obtained by taking a scale-selective approach whereby the precision of variables is gradually decreased at smaller spatial scales to optimise the overall efficiency of the model. To study the effect of reducing precision to different levels on multiple spatial scales, we here introduce a new model atmosphere developed by extending the Lorenz '96 idealised system to encompass three tiers of variables - which represent large-, medium- and small-scale features - for the first time. In this chaotic but computationally tractable system, the 'true' state can be defined by explicitly resolving all three tiers. The abilities of low resolution (single-tier) double-precision models and similar-cost high resolution (two-tier) models in mixed-precision to produce accurate forecasts of this 'truth' are compared. The high resolution models outperform the low resolution ones even when small-scale variables are resolved in half-precision (16 bits). This suggests that using scale-dependent levels of precision in more complicated real-world Earth System models could allow forecasts to be made at higher resolution and with improved accuracy. If adopted, this new paradigm would represent a revolution in numerical modelling that could be of great benefit to the world.
Resolving the neutron lifetime puzzle
NASA Astrophysics Data System (ADS)
Mumm, Pieter
2018-05-01
Free electrons and protons are stable, but outside atomic nuclei, free neutrons decay into a proton, electron, and antineutrino through the weak interaction, with a lifetime of ∼880 s (see the figure). The most precise measurements have stated uncertainties below 1 s (0.1%), but different techniques, although internally consistent, disagree by 4 standard deviations given the quoted uncertainties. Resolving this “neutron lifetime puzzle” has spawned much experimental effort as well as exotic theoretical mechanisms, thus far without a clear explanation. On page 627 of this issue, Pattie et al. (1) present the most precise measurement of the neutron lifetime to date. A new method of measuring trapped neutrons in situ allows a more detailed exploration of one of the more pernicious systematic effects in neutron traps, neutron phase-space evolution (the changing orbits of neutrons in the trap), than do previous methods. The precision achieved, combined with a very different set of systematic uncertainties, gives hope that experiments such as this one can help resolve the current situation with the neutron lifetime.
Recent trends in spin-resolved photoelectron spectroscopy
NASA Astrophysics Data System (ADS)
Okuda, Taichi
2017-12-01
Since the discovery of the Rashba effect on crystal surfaces and also the discovery of topological insulators, spin- and angle-resolved photoelectron spectroscopy (SARPES) has become more and more important, as the technique can measure directly the electronic band structure of materials with spin resolution. In the same way that the discovery of high-Tc superconductors promoted the development of high-resolution angle-resolved photoelectron spectroscopy, the discovery of this new class of materials has stimulated the development of new SARPES apparatus with new functions and higher resolution, such as spin vector analysis, ten times higher energy and angular resolution than conventional SARPES, multichannel spin detection, and so on. In addition, the utilization of vacuum ultra violet lasers also opens a pathway to the realization of novel SARPES measurements. In this review, such recent trends in SARPES techniques and measurements will be overviewed.
NASA Astrophysics Data System (ADS)
Bromberger, H.; Ermolov, A.; Belli, F.; Liu, H.; Calegari, F.; Chávez-Cervantes, M.; Li, M. T.; Lin, C. T.; Abdolvand, A.; Russell, P. St. J.; Cavalleri, A.; Travers, J. C.; Gierz, I.
2015-08-01
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.
Manufacturing Technology Development of Advanced Components for High Power Solid State Lasers
2010-07-19
commercially available that can support an intra-cavity wavelength of 1030 nm. Losses were reduced by ensuring that the apex angle provided a Brewster ...in Figure 2.2), one can map the optical path distance distribution near the interface region. An oblique angle may be used to resolve the order of...U:YAG) composite of a 62° incident angle in (A), and a .5% Er:YAG// U:YAG composite of a 20° incident angle in (B) The refractive index difference
The Development of using the digital projection method to measure the contact angle of ball screw
NASA Astrophysics Data System (ADS)
Chen, Chun-Jen; Jywe, Wenyuh; Liu, Yu-Chun; Jwo, Hsin-Hong
The ball screw frequently used to drive or translate the parts on the precision machine, such as machine tool and motorized stage. Therefore they were most frequently used on the precision machine, semiconductor equipment, medical instrument and aero industry. The main parts of ball screw are screw, ball and nut. The contact angle between the screw, ball and nut will affect the performance (include loading and noise) and lifecycle of a ball screw. If the actual contact angle and the designed contact angle are not the same, the friction between the ball, screw and nut will increase and it will result in the thermal increase and lifecycle decrease. This paper combines the traditional profile projector and commercial digital camera to build an imaging based and noncontact measurements system. It can implement the contact angle measurement quickly and accurately. Three different pitch angles of ball screws were completed tests in this paper. The angle resolution of this measurement system is about 0.001 degree and its accuracy is about 0.05 degree.
Gao, Song; Lee, Sang-Shin; Kim, Eun-Soo; Choi, Duk-Yong
2018-06-21
An optical device with minimized dimensions, which is capable of efficiently resolving an ultra-broad spectrum into a wide splitting angle but incurring no spectrum overlap, is of importance in advancing the development of spectroscopy. Unfortunately, this challenging task cannot be easily addressed through conventional geometrical or diffractive optical elements. Herein, we propose and demonstrate vertically integrated visible and near-infrared metasurfaces which render an ultra-broadband and highly angle-resolved anomalous reflection. The proposed metasurface capitalizes on a supercell that comprises two vertically concatenated trapezoid-shaped aluminum antennae, which are paired with a metallic ground plane via a dielectric layer. Under normal incidence, reflected light within a spectral bandwidth of 1000 nm ranging from λ = 456 nm to 1456 nm is efficiently angle-resolved to a single diffraction order with no spectrum overlap via the anomalous reflection, exhibiting an average reflection efficiency over 70% and a substantial angular splitting of 58°. In light of a supercell pitch of 1500 nm, to the best of our knowledge, the micron-scale bandwidth is the largest ever reported. It is noted that the substantially wide bandwidth has been accomplished by taking advantage of spectral selective vertical coupling effects between antennae and ground plane. In the visible regime, the upper antenna primarily renders an anomalous reflection by cooperating with the lower antenna, which in turn cooperates with the ground plane and produces phase variations leading to an anomalous reflection in the near-infrared regime. Misalignments between the two antennae have been particularly inspected to not adversely affect the anomalous reflection, thus guaranteeing enhanced structural tolerance of the proposed metasurface.
Machining of Silicon-Ribbon-Forming Dies
NASA Technical Reports Server (NTRS)
Menna, A. A.
1985-01-01
Carbon extension for dies used in forming silicon ribbon crystals machined precisely with help of special tool. Die extension has edges beveled toward narrow flats at top, with slot precisely oriented and centered between flats and bevels. Cutting tool assembled from standard angle cutter and circular saw or saws. Angle cutters cuts bevels while slot saw cuts slot between them. In alternative version, custom-ground edges or additional circular saws also cut flats simultaneously.
Alania, M; Lobato, I; Van Aert, S
2018-01-01
In this paper, both the frozen lattice (FL) and the absorptive potential (AP) approximation models are compared in terms of the integrated intensity and the precision with which atomic columns can be located from an image acquired using high angle annular dark field (HAADF) scanning transmission electron microscopy (STEM). The comparison is made for atoms of Cu, Ag, and Au. The integrated intensity is computed for both an isolated atomic column and an atomic column inside an FCC structure. The precision has been computed using the so-called Cramér-Rao Lower Bound (CRLB), which provides a theoretical lower bound on the variance with which parameters can be estimated. It is shown that the AP model results into accurate measurements for the integrated intensity only for small detector ranges under relatively low angles and for small thicknesses. In terms of the attainable precision, both methods show similar results indicating picometer range precision under realistic experimental conditions. Copyright © 2017 Elsevier B.V. All rights reserved.
NASA Astrophysics Data System (ADS)
Gotlieb, K.; Hussain, Z.; Bostwick, A.; Lanzara, A.; Jozwiak, C.
2013-09-01
A high-efficiency spin- and angle-resolved photoemission spectroscopy (spin-ARPES) spectrometer is coupled with a laboratory-based laser for rapid high-resolution measurements. The spectrometer combines time-of-flight (TOF) energy measurements with low-energy exchange scattering spin polarimetry for high detection efficiencies. Samples are irradiated with fourth harmonic photons generated from a cavity-dumped Ti:sapphire laser that provides high photon flux in a narrow bandwidth, with a pulse timing structure ideally matched to the needs of the TOF spectrometer. The overall efficiency of the combined system results in near-EF spin-resolved ARPES measurements with an unprecedented combination of energy resolution and acquisition speed. This allows high-resolution spin measurements with a large number of data points spanning multiple dimensions of interest (energy, momentum, photon polarization, etc.) and thus enables experiments not otherwise possible. The system is demonstrated with spin-resolved energy and momentum mapping of the L-gap Au(111) surface states, a prototypical Rashba system. The successful integration of the spectrometer with the pulsed laser system demonstrates its potential for simultaneous spin- and time-resolved ARPES with pump-probe based measurements.
Test technology on divergence angle of laser range finder based on CCD imaging fusion
NASA Astrophysics Data System (ADS)
Shi, Sheng-bing; Chen, Zhen-xing; Lv, Yao
2016-09-01
Laser range finder has been equipped with all kinds of weapons, such as tank, ship, plane and so on, is important component of fire control system. Divergence angle is important performance and incarnation of horizontal resolving power for laser range finder, is necessary appraised test item in appraisal test. In this paper, based on high accuracy test on divergence angle of laser range finder, divergence angle test system is designed based on CCD imaging, divergence angle of laser range finder is acquired through fusion technology for different attenuation imaging, problem that CCD characteristic influences divergence angle test is solved.
Zhao, Jing-Xin; Su, Xiu-Yun; Xiao, Ruo-Xiu; Zhao, Zhe; Zhang, Li-Hai; Zhang, Li-Cheng; Tang, Pei-Fu
2016-11-01
We established a mathematical method to precisely calculate the radiographic anteversion (RA) and radiographic inclination (RI) angles of the acetabular cup based on anterior-posterior (AP) pelvic radiographs after total hip arthroplasty. Using Mathematica software, a mathematical model for an oblique cone was established to simulate how AP pelvic radiographs are obtained and to address the relationship between the two-dimensional and three-dimensional geometry of the opening circle of the cup. In this model, the vertex was the X-ray beam source, and the generatrix was the ellipse in radiographs projected from the opening circle of the acetabular cup. Using this model, we established a series of mathematical formulas to reveal the differences between the true RA and RI cup angles and the measurements results achieved using traditional methods and AP pelvic radiographs and to precisely calculate the RA and RI cup angles based on post-operative AP pelvic radiographs. Statistical analysis indicated that traditional methods should be used with caution if traditional measurements methods are used to calculate the RA and RI cup angles with AP pelvic radiograph. The entire calculation process could be performed by an orthopedic surgeon with mathematical knowledge of basic matrix and vector equations. Copyright © 2016 IPEM. Published by Elsevier Ltd. All rights reserved.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Harak, B. A. de; Bartschat, K.; Martin, N. L. S.
Angular distribution and spectral (e,2e) measurements are reported for the helium autoionizing levels (2s{sup 2}){sup 1}S, (2p{sup 2}){sup 1}D, and (2s2p){sup 1}P. A special out-of-plane geometry is used where the ejected electrons are emitted in a plane perpendicular to the scattered electron direction. The kinematics are chosen so that this plane contains the momentum-transfer direction. While the recoil peak almost vanishes in the angular distribution for direct ionization, it remains significant for the autoionizing levels and exhibits a characteristic shape for each orbital angular momentum L=0,1,2. A second-order model in the projectile-target interaction correctly reproduces the observed magnitudes of themore » recoil peaks, but is a factor of 2 too large in the central out-of-plane region. Observed (e,2e) energy spectra for the three resonances over the full angular range are well reproduced by the second-order calculation. Calculations using a first-order model fail to reproduce both the magnitudes of the recoil peaks and the spectral line profiles.« less
Collective relaxation processes in atoms, molecules and clusters
NASA Astrophysics Data System (ADS)
Kolorenč, Přemysl; Averbukh, Vitali; Feifel, Raimund; Eland, John
2016-04-01
Electron correlation is an essential driver of a variety of relaxation processes in excited atomic and molecular systems. These are phenomena which often lead to autoionization typically involving two-electron transitions, such as the well-known Auger effect. However, electron correlation can give rise also to higher-order processes characterized by multi-electron transitions. Basic examples include simultaneous two-electron emission upon recombination of an inner-shell vacancy (double Auger decay) or collective decay of two holes with emission of a single electron. First reports of this class of processes date back to the 1960s, but their investigation intensified only recently with the advent of free-electron lasers. High fluxes of high-energy photons induce multiple excitation or ionization of a system on the femtosecond timescale and under such conditions the importance of multi-electron processes increases significantly. We present an overview of experimental and theoretical works on selected multi-electron relaxation phenomena in systems of different complexity, going from double Auger decay in atoms and small molecules to collective interatomic autoionization processes in nanoscale samples.
Synchrotron-based valence shell photoionization of CH radical
DOE Office of Scientific and Technical Information (OSTI.GOV)
Gans, B., E-mail: berenger.gans@u-psud.fr, E-mail: christian.alcaraz@u-psud.fr; Falvo, C.; Holzmeier, F.
2016-05-28
We report the first experimental observations of X{sup +} {sup 1}Σ{sup +}←X {sup 2}Π and a{sup +} {sup 3}Π←X {sup 2}Π single-photon ionization transitions of the CH radical performed on the DESIRS beamline at the SOLEIL synchrotron facility. The radical was produced by successive hydrogen-atom abstractions on methane by fluorine atoms in a continuous microwave discharge flow tube. Mass-selected ion yields and photoelectron spectra were recorded as a function of photon energy using a double imaging photoelectron/photoion coincidence spectrometer. The ion yield appears to be strongly affected by vibrational and electronic autoionizations, which allow the observation of high Rydberg statesmore » of the neutral species. The photoelectron spectra enable the first direct determinations of the adiabatic ionization potential and the energy of the first triplet state of the cation with respect to its singlet ground state. This work also brings valuable information on the complex electronic structure of the CH radical and its cation and adds new observations to complement our understanding of Rydberg states and autoionization processes.« less
Electron-impact Ionization of P-like Ions Forming Si-like Ions
NASA Astrophysics Data System (ADS)
Kwon, D.-H.; Savin, D. W.
2014-03-01
We have calculated electron-impact ionization (EII) for P-like systems from P to Zn15 + forming Si-like ions. The work was performed using the flexible atomic code (FAC) which is based on a distorted-wave approximation. All 3l → nl' (n = 3-35) excitation-autoionization (EA) channels near the 3p direct ionization threshold and 2l → nl' (n = 3-10) EA channels at the higher energies are included. Close attention has been paid to the detailed branching ratios. Our calculated total EII cross sections are compared both with previous FAC calculations, which omitted many of these EA channels, and with the available experimental results. Moreover, for Fe11 +, we find that part of the remaining discrepancies between our calculations and recent measurements can be accounted for by the inclusion of the resonant excitation double autoionization process. Lastly, at the temperatures where each ion is predicted to peak in abundances in collisional ionization equilibrium, the Maxwellian rate coefficients derived from our calculations differ by 50%-7% from the previous FAC rate coefficients, with the difference decreasing with increasing charge.
77 FR 10693 - Airworthiness Directives; Airbus Airplanes
Federal Register 2010, 2011, 2012, 2013, 2014
2012-02-23
... the position resolvers of the angle of attack (AOA) vane, which was a result of incorrect removal of... non-activation of the AOA protection systems which, during flight at a high angle of attack, could... information identified in this proposed AD, contact Airbus, Airworthiness Office--EAS, 1 Rond Point Maurice...
Numerical Aspects of Atomic Physics: Helium Basis Sets and Matrix Diagonalization
NASA Astrophysics Data System (ADS)
Jentschura, Ulrich; Noble, Jonathan
2014-03-01
We present a matrix diagonalization algorithm for complex symmetric matrices, which can be used in order to determine the resonance energies of auto-ionizing states of comparatively simple quantum many-body systems such as helium. The algorithm is based in multi-precision arithmetic and proceeds via a tridiagonalization of the complex symmetric (not necessarily Hermitian) input matrix using generalized Householder transformations. Example calculations involving so-called PT-symmetric quantum systems lead to reference values which pertain to the imaginary cubic perturbation (the imaginary cubic anharmonic oscillator). We then proceed to novel basis sets for the helium atom and present results for Bethe logarithms in hydrogen and helium, obtained using the enhanced numerical techniques. Some intricacies of ``canned'' algorithms such as those used in LAPACK will be discussed. Our algorithm, for complex symmetric matrices such as those describing cubic resonances after complex scaling, is faster than LAPACK's built-in routines, for specific classes of input matrices. It also offer flexibility in terms of the calculation of the so-called implicit shift, which is used in order to ``pivot'' the system toward the convergence to diagonal form. We conclude with a wider overview.
A rotationally biased upwind difference scheme for the Euler equations
NASA Technical Reports Server (NTRS)
Davis, S. F.
1983-01-01
The upwind difference schemes of Godunov, Osher, Roe and van Leer are able to resolve one dimensional steady shocks for the Euler equations within one or two mesh intervals. Unfortunately, this resolution is lost in two dimensions when the shock crosses the computing grid at an oblique angle. To correct this problem, a numerical scheme was developed which automatically locates the angle at which a shock might be expected to cross the computing grid and then constructs separate finite difference formulas for the flux components normal and tangential to this direction. Numerical results which illustrate the ability of this method to resolve steady oblique shocks are presented.
Time-resolved coherent X-ray diffraction imaging of surface acoustic waves
Nicolas, Jan-David; Reusch, Tobias; Osterhoff, Markus; Sprung, Michael; Schülein, Florian J. R.; Krenner, Hubert J.; Wixforth, Achim; Salditt, Tim
2014-01-01
Time-resolved coherent X-ray diffraction experiments of standing surface acoustic waves, illuminated under grazing incidence by a nanofocused synchrotron beam, are reported. The data have been recorded in stroboscopic mode at controlled and varied phase between the acoustic frequency generator and the synchrotron bunch train. At each time delay (phase angle), the coherent far-field diffraction pattern in the small-angle regime is inverted by an iterative algorithm to yield the local instantaneous surface height profile along the optical axis. The results show that periodic nanoscale dynamics can be imaged at high temporal resolution in the range of 50 ps (pulse length). PMID:25294979
Lo Vecchio, I; Denlinger, J D; Krupin, O; Kim, B J; Metcalf, P A; Lupi, S; Allen, J W; Lanzara, A
2016-10-14
Using angle resolved photoemission spectroscopy, we report the first band dispersions and distinct features of the bulk Fermi surface (FS) in the paramagnetic metallic phase of the prototypical metal-insulator transition material V_{2}O_{3}. Along the c axis we observe both an electron pocket and a triangular holelike FS topology, showing that both V 3d a_{1g} and e_{g}^{π} states contribute to the FS. These results challenge the existing correlation-enhanced crystal field splitting theoretical explanation for the transition mechanism and pave the way for the solution of this mystery.
Time-resolved coherent X-ray diffraction imaging of surface acoustic waves.
Nicolas, Jan-David; Reusch, Tobias; Osterhoff, Markus; Sprung, Michael; Schülein, Florian J R; Krenner, Hubert J; Wixforth, Achim; Salditt, Tim
2014-10-01
Time-resolved coherent X-ray diffraction experiments of standing surface acoustic waves, illuminated under grazing incidence by a nanofocused synchrotron beam, are reported. The data have been recorded in stroboscopic mode at controlled and varied phase between the acoustic frequency generator and the synchrotron bunch train. At each time delay (phase angle), the coherent far-field diffraction pattern in the small-angle regime is inverted by an iterative algorithm to yield the local instantaneous surface height profile along the optical axis. The results show that periodic nanoscale dynamics can be imaged at high temporal resolution in the range of 50 ps (pulse length).
DOE Office of Scientific and Technical Information (OSTI.GOV)
Heinemann, Thomas, E-mail: thomas.heinemann@tu-berlin.de; Klapp, Sabine H. L., E-mail: klapp@physik.tu-berlin.de; Palczynski, Karol, E-mail: karol.palczynski@helmholtz-berlin.de
We present an approach for calculating coarse-grained angle-resolved effective pair potentials for uniaxial molecules. For integrating out the intramolecular degrees of freedom we apply umbrella sampling and steered dynamics techniques in atomistically-resolved molecular dynamics (MD) computer simulations. Throughout this study we focus on disk-like molecules such as coronene. To develop the methods we focus on integrating out the van der Waals and intramolecular interactions, while electrostatic charge contributions are neglected. The resulting coarse-grained pair potential reveals a strong temperature and angle dependence. In the next step we fit the numerical data with various Gay-Berne-like potentials to be used in moremore » efficient simulations on larger scales. The quality of the resulting coarse-grained results is evaluated by comparing their pair and many-body structure as well as some thermodynamic quantities self-consistently to the outcome of atomistic MD simulations of many-particle systems. We find that angle-resolved potentials are essential not only to accurately describe crystal structures but also for fluid systems where simple isotropic potentials start to fail already for low to moderate packing fractions. Further, in describing these states it is crucial to take into account the pronounced temperature dependence arising in selected pair configurations due to bending fluctuations.« less
Where is your arm? Variations in proprioception across space and tasks.
Fuentes, Christina T; Bastian, Amy J
2010-01-01
The sense of limb position is crucial for movement control and environmental interactions. Our understanding of this fundamental proprioceptive process, however, is limited. For example, little is known about the accuracy of arm proprioception: Does it vary with changes in arm configuration, since some peripheral receptors are engaged only when joints move toward extreme angles? Are these variations consistent across different tasks? Does proprioceptive ability change depending on what we try to localize (e.g., fingertip position vs. elbow angle)? We used a robot exoskeleton to study proprioception in 14 arm configurations across three tasks, asking healthy subjects to 1) match a pointer to elbow angles after passive movements, 2) match a pointer to fingertip positions after passive movements, and 3) actively match their elbow angle to a pointer. Across all three tasks, subjects overestimated more extreme joint positions; this may be due to peripheral sensory signals biasing estimates as a safety mechanism to prevent injury. We also found that elbow angle estimates were more precise when used to judge fingertip position versus directly reported, suggesting that the brain has better access to limb endpoint position than joint angles. Finally, precision of elbow angle estimates improved in active versus passive movements, corroborating work showing that efference copies of motor commands and alpha-gamma motor neuron coactivation contribute to proprioceptive estimates. In sum, we have uncovered fundamental aspects of normal proprioceptive processing, demonstrating not only predictable biases that are dependent on joint configuration and independent of task but also improved precision when integrating information across joints.
Bullet trajectory reconstruction - Methods, accuracy and precision.
Mattijssen, Erwin J A T; Kerkhoff, Wim
2016-05-01
Based on the spatial relation between a primary and secondary bullet defect or on the shape and dimensions of the primary bullet defect, a bullet's trajectory prior to impact can be estimated for a shooting scene reconstruction. The accuracy and precision of the estimated trajectories will vary depending on variables such as, the applied method of reconstruction, the (true) angle of incidence, the properties of the target material and the properties of the bullet upon impact. This study focused on the accuracy and precision of estimated bullet trajectories when different variants of the probing method, ellipse method, and lead-in method are applied on bullet defects resulting from shots at various angles of incidence on drywall, MDF and sheet metal. The results show that in most situations the best performance (accuracy and precision) is seen when the probing method is applied. Only for the lowest angles of incidence the performance was better when either the ellipse or lead-in method was applied. The data provided in this paper can be used to select the appropriate method(s) for reconstruction and to correct for systematic errors (accuracy) and to provide a value of the precision, by means of a confidence interval of the specific measurement. Copyright © 2016 Elsevier Ireland Ltd. All rights reserved.
NASA Astrophysics Data System (ADS)
Fontaine, Norman Henry
1997-10-01
Techniques which can be used to obtain depth-resolved information on the thermodynamics at polymer-polymer and polymer-wall interfaces, and of small molecule diffusion in polymers, are of particular interest to industry. Optical methods which are sensitive to molecular vibrations (such as internal reflection Raman spectroscopy) are advantageous because they can non- destructively probe molecular content, orientation, and polarity of the local environment in a sample. However, while optical internal reflection depth-profiling methods have been reported, they have never progressed beyond the demonstration stage. In this work, the theory and methodology of internal reflection spectroscopy are developed and optimized into a rigorous field-controlled spectroscopic technique. A novel asymmetric internal reflection element (IRE) is introduced which traps back-reflections, allowing precise evanescent and standing wave probe-field control in the sample for all angles of incidence. It is demonstrated that a Gaussian laser beam will best approximate an infinite homogeneous plane wave when the IRE/sample interface lies in the paraxial-Fraunhofer region (far- field) of the beam path. Calibration methods are presented, sources of systematic errors are identified, and the angular resolution limit (ARL) is introduced as a measure of the field control developed in a sample by any internal reflection method. A general model of Raman scattering and photon detection from multi-layer thin films is developed. A new and generalized operator based transfer matrix method is developed and applied to electromagnetic field and diffusion computations in multi-layer systems. Total internal reflection spectroscopy is extended to include sub-critical angles of incidence, where resonant field enhancements generate large and selective amplification of the probe-field intensity within the layers of the sample. Fitting these resonances to the model spectral intensities allows unique determination of the location of buried interfaces in micron-sized polymer multi-layers with nanometer scale precision and the refractive indices of the layers with precision of /Delta n/approx/pm 0.0001. The Raman active molecular content of each optically distinct layer of the film is determinable simultaneously with the optical properties. Resonant mode VAIRRS studies of poly(methyl methacrylate) films spun-cast from toluene and then dried under ambient conditions have shown evidence for toluene diffusion concurrent with a rotationally hindered relaxation of oriented ester side groups about the polymer backbone. Low temperature annealing (≈87oC) has shown evidence that this hindered rotational relaxation may be reversible. VAIRRS study of a polystyrene/poly(methyl methacrylate) bi-layer has detected evidence for toluene diffusion across the buried polymer-polymer interface.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Bromberger, H., E-mail: Hubertus.Bromberger@mpsd.mpg.de; Liu, H.; Chávez-Cervantes, M.
2015-08-31
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi{sub 2}Se{sub 3} with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz,more » with photon energies that cover the first Brillouin zone of most materials.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Safronova, U.I.; Safronova, A.S.; Beiersdorfer, P.
Energy levels, radiative transition probabilities, and autoionization rates for 1s{sup 2}2s{sup 2}2p{sup 5}3l{sup '}nl,1s{sup 2}2s2p{sup 6}3l{sup '}nl(n=3-7,l{<=}n-1) and 1s{sup 2}2s{sup 2}2p{sup 5}4l{sup '}nl,1s{sup 2}2s2p{sup 6}4l{sup '}nl(n=4-6,l{<=}n-1) states in Na-like tungsten (W{sup 63+}) are calculated. Cowan's relativistic Hartree-Fock method, the relativistic multiconfiguration method implemented in the Hebrew University Lawrence Livermore Atomic Code, and the relativistic many-body perturbation theory method, are used. Autoionizing levels above the threshold 1s{sup 2}2s{sup 2}2p{sup 6} are considered. It is found that configuration mixing [3sns+3pnp+3dnd],[3snp+3pns+3pnd+3dnp] plays an important role for all atomic characteristics. Also strong mixing between states with 2s and 2p holes (1s{sup 2}2s{sup 2}2p{sup 5}3l{submore » 1}nl{sub 2}+1s{sup 2}2s2p{sup 6}3l{sub 3}nl{sub 4}) occurs. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and dielectronic recombination (DR) rate coefficients are determined for the excited 1s{sup 2}2s{sup 2}2p{sup 6}nl(n=3-7,l{<=}n-1) states. It is shown that the contribution of the highly excited states is very important for calculation of total DR rates. Contributions from the autoionizing states 1s{sup 2}2s{sup 2}2p{sup 5}3l{sup '}nl,1s{sup 2}2s2p{sup 6}3l{sup '}nl(n{>=}8) and 1s{sup 2}2s{sup 2}2p{sup 5}4l{sup '}nl,1s{sup 2}2s2p{sup 6}4l{sup '}nl(n{>=}7) to the DR rate coefficients are estimated by extrapolation of all atomic parameters. The orbital angular momentum (l) distribution of the rate coefficients shows a peak at l=2. The total DR rate coefficient is derived as a function of electron temperature. The dielectronic satellite spectra of W{sup 63+} are important for L-shell diagnostics of very high-temperature laboratory plasmas such as future ITER fusion plasmas.« less
Influence of the air’s refractive index on precision angle metrology with autocollimators
NASA Astrophysics Data System (ADS)
Geckeler, Ralf D.; Křen, Petr; Just, Andreas; Schumann, Matthias; Krause, Michael
2018-07-01
In this paper, we discuss a substantial—though previously neglected—error source in precision metrology with autocollimators, specifically, changes in the air’s refractive index, with a focus on the dominant impact of pressure changes. Pressure decreases with increasing elevation above sea level and is subject to substantial variation due to weather changes. It causes changes in an autocollimator’s angle response which are proportional to the measured angle and which increase linearly with the beam length and air pressure. We characterise this important influence in detail by using extended theoretical and experimental investigations and derive strategies for correcting it. We discuss its implications for the comparison of autocollimator calibrations performed at different metrology institutes which is crucial for validating their calibration capabilities. This work aims at approaching fundamental limits in angle metrology with autocollimators.
NASA Technical Reports Server (NTRS)
Barker, L. Keith; Mckinney, William S., Jr.
1989-01-01
The Laboratory Telerobotic Manipulator (LTM) is a seven-degree-of-freedom robot arm. Two of the arms were delivered to Langley Research Center for ground-based research to assess the use of redundant degree-of-freedom robot arms in space operations. Resolved-rate control equations for the LTM are derived. The equations are based on a scheme developed at the Oak Ridge National Laboratory for computing optimized joint angle rates in real time. The optimized joint angle rates actually represent a trade-off, as the hand moves, between small rates (least-squares solution) and those rates which work toward satisfying a specified performance criterion of joint angles. In singularities where the optimization scheme cannot be applied, alternate control equations are devised. The equations developed were evaluated using a real-time computer simulation to control a 3-D graphics model of the LTM.
Novel Tiltmeter for Monitoring Angle Shift In Incident Waves
2008-12-01
40th Annual Precise Time and Time Interval (PTTI) Meeting 559 NOVEL TILTMETER FOR MONITORING ANGLE SHIFT IN INCIDENT WAVES S... Tiltmeter For Monitoring Angle Shift In Incident Waves 5a. CONTRACT NUMBER 5b. GRANT NUMBER 5c. PROGRAM ELEMENT NUMBER 6. AUTHOR(S) 5d. PROJECT...up, any angle change of the incident beam ’θ results in a change of the intensity transmission of the resonator. A NOVEL ANGLE TILTMETER
Spherical grating monochromator with interferometer control and in-vacuum reference
NASA Astrophysics Data System (ADS)
Holly, D. J.; Mason, W. P.; Sailor, T.; Smith, R. E.; Wahl, D.
2002-03-01
Physical Science Laboratory's new generation of spherical grating monochromators incorporates a laser interferometer to control scan angle and an in-vacuum absolute angle reference, as well as other improvements. The design accommodates up to six gratings which can be moved axially (under motor control, with encoder position readback) at any scan angle. The gratings are cooled by means of spring-loaded clamps which conduct heat to a water-cooled plate. The instruments feature hollow roller bearings on the scan axis to minimize bearing runout, and a pseudosine-bar drive for precise control of grating angle. The interferometer angle-measuring optics are mounted inside the vacuum chamber and measure the angle between the grating scan axis and the instrument's granite base. The laser interferometer measures the grating angle with a resolution of approximately 0.02 arcsec over the entire scan range of 40°. To provide a reference for the interferometer angle measurement, we have built an in-vacuum optical reference which uses custom chrome-on-glass reticles mounted inside the vacuum chamber. Collimated light from a source outside the vacuum passes through the reticles to yield quadrature signals which precisely define an absolute reference angle for the interferometer. Repeatability of the grating angle is within a range of ±0.05 arcsec. Two of these instruments are in operation at SRRC (Taiwan) and a third instrument has been delivered to NSLS (Brookhaven).
Detection of a poorly resolved airplane using SWIR polarization imaging
NASA Astrophysics Data System (ADS)
Dahl, Laura M.; Shaw, Joseph A.; Chenault, David B.
2016-05-01
Polarization can be used to detect manmade objects on the ground and in the air, as it provides additional information beyond intensity and color. Skylight can be strongly polarized, so the detection of airplanes in flight requires careful consideration of the skylight degree and angle of polarization (DoLP, AoP). In this study, we detect poorly resolved airplanes (>= 4 pixels on target) in flight during daytime partly cloudy and smoky conditions in Bozeman, Montana. We used a Polaris Sensor Technologies SWIR-MWIR rotating imaging polarimeter to measure the polarization signatures of airplanes and the surrounding skylight from 1.5 to 1.8 μm in the short-wave infrared (SWIR). An airplane flying in a clear region of partly cloudy sky was found to be 69% polarized at an elevation angle of 13° with respect to the horizon and the surrounding skylight was 4-8% polarized (maximum skylight DoLP was found to be 7-14% at an elevation angle of 50°). As the airplane increased in altitude, the DoLP for both airplane and surrounding sky pixels increased as the airplane neared the band of maximum sky polarization. We also observed that an airplane can be less polarized than its surrounding skylight when there is heavy smoke present. In such a case, the airplane was 30-38% polarized at an elevation angle of 17°, while the surrounding skylight was approximately 40% polarized (maximum skylight DoLP was 40-55% at an elevation angle of 34°). In both situations the airplane was most consistently observed in DoLP images rather than S0 or AoP images. In this paper, we describe the results in detail and discuss how this phenomenology could detect barely resolved aircrafts.
Angle-resolved photoluminescence spectrum of a uniform phosphor layer
NASA Astrophysics Data System (ADS)
Fujieda, Ichiro; Ohta, Masamichi
2017-10-01
A photoluminescence spectrum depends on an emission angle due to self-absorption in a phosphor material. Assuming isotropic initial emission and Lambert-Beer's law, we have derived simple expressions for the angle-resolved spectra emerging from the top and bottom surfaces of a uniform phosphor layer. The transmittance of an excitation light through the phosphor layer can be regarded as a design parameter. For a strongly-absorbing phosphor layer, the forward flux is less intense and more red-shifted than the backward flux. The red-shift is enhanced as the emission direction deviates away from the plane normal. When we increase the transmittance, the backward flux decreases monotonically. The forward flux peaks at a certain transmittance value. The two fluxes become similar to each other for a weakly-absorbing phosphor layer. We have observed these behaviors in experiment. In a practical application, self-absorption decreases the efficiency of conversion and results in angle-dependent variations in chromaticity coordinates. A patterned phosphor layer with a secondary optical element such as a remote reflector alleviates these problems.
The theory precision analyse of RFM localization of satellite remote sensing imagery
NASA Astrophysics Data System (ADS)
Zhang, Jianqing; Xv, Biao
2009-11-01
The tradition method of detecting precision of Rational Function Model(RFM) is to make use of a great deal check points, and it calculates mean square error through comparing calculational coordinate with known coordinate. This method is from theory of probability, through a large number of samples to statistic estimate value of mean square error, we can think its estimate value approaches in its true when samples are well enough. This paper is from angle of survey adjustment, take law of propagation of error as the theory basis, and it calculates theory precision of RFM localization. Then take the SPOT5 three array imagery as experiment data, and the result of traditional method and narrated method in the paper are compared, while has confirmed tradition method feasible, and answered its theory precision question from the angle of survey adjustment.
The MINOS Experiment: Results and Prospects
Evans, J. J.
2013-01-01
Tmore » he MINOS experiment has used the world’s most powerful neutrino beam to make precision neutrino oscillation measurements. By observing the disappearance of muon neutrinos, MINOS has made the world’s most precise measurement of the larger neutrino mass splitting and has measured the neutrino mixing angle θ 23 . Using a dedicated antineutrino beam, MINOS has made the first direct precision measurements of the corresponding antineutrino parameters. A search for ν e and ν - e appearance has enabled a measurement of the mixing angle θ 13 . A measurement of the neutral-current interaction rate has confirmed oscillation between three active neutrino flavours. MINOS will continue as MINOS+ in an upgraded beam with higher energy and intensity, allowing precision tests of the three-flavour neutrino oscillation picture, in particular a very sensitive search for the existence of sterile neutrinos.« less
Photon Doppler velocimetry measurements of transverse surface velocities
NASA Astrophysics Data System (ADS)
Johnson, C. R.; LaJeunesse, J. W.; Sable, P. A.; Dawson, A.; Hatzenbihler, A.; Borg, J. P.
2018-06-01
The goal of this work was to develop a technique for making transverse surface velocity measures utilizing Photon Doppler Velocimetry (PDV). Such a task is achieved by transmitting light and collecting Doppler-shifted light at an angle relative to the normal axis, where measured velocities are representative of a component of the transverse velocity. Because surface characteristics have an intrinsic effect on light scatter, different surface preparations were explored to direct reflectivity, including diffusion by means of sandpapering, or increasing retroreflectivity by coating with microspheres, milling v-cuts, and electrochemically etching grooves. Testing of these surface preparations was performed using an experiment featuring a 30 mm diameter aluminum disk rotating at 6000 or 6600 RPM. A single PDV collimator was positioned along the rotational axis of the disk at various angles, resolving the apparent transverse velocity. To characterize surface preparations, light return and velocities were recorded as a function of probe angle ranging from 0° to 51° from the surface normal for each preparation. Polished and electrochemically etched surfaces did not provide enough reflected light to resolve a beat frequency; however, sandpapered surfaces, retroreflective microspheres, and milled v-cuts provided adequate reflected light for incidence angles up to 51°. Applications of the surface preparations were then studied in gas gun experiments. Retroreflective microspheres were studied in a planar impact experiment, and milled v-cuts were studied in an oblique impact experiment. A normal and transverse profile of particle velocity was resolved in the oblique impact experiment.
Direct, experimental evidence of the Fermi surface in YBa2Cu3O(7-x)
NASA Astrophysics Data System (ADS)
Haghighi, H.; Kaiser, J. H.; Rayner, S. L.; West, R. N.; Liu, J. Z.; Shelton, R.; Howell, R. H.; Sterne, P. A.; Solal, F. R.; Fluss, M. J.
1991-04-01
We report new measurements of the electron positron momentum spectra of YBa2Cu3O(7-x) performed with ultra-high statistical precision. These data differ from previous results in two significant respects: They show the D(sub 2) symmetry appropriate for untwinned crystals and, more importantly, they show unmistakable, statistically significant, discontinuities that are evidence of a major Fermi surface section. These results provide a partial answer to a question of special significance to the study of high temperature superconductors i.e., the distribution of the electrons in the material, the electronic structure. Special consideration has been given both experimentally and theoretically to the existence and shape of a Fermi surface in the materials and to the superconducting gap. There are only three experimental techniques that can provide details of the electronic structure at useful resolutions. They are angular correlation of positron annihilation radiation, ACAR, angle resolved photo emission, PE, and de Haas van Alphen measurements.
Distribution of Plasmoids in Post-Coronal Mass Ejection Current Sheets
NASA Astrophysics Data System (ADS)
Bhattacharjee, A.; Guo, L.; Huang, Y.
2013-12-01
Recently, the fragmentation of a current sheet in the high-Lundquist-number regime caused by the plasmoid instability has been proposed as a possible mechanism for fast reconnection. In this work, we investigate this scenario by comparing the distribution of plasmoids obtained from Large Angle and Spectrometric Coronagraph (LASCO) observational data of a coronal mass ejection event with a resistive magnetohydrodynamic simulation of a similar event. The LASCO/C2 data are analyzed using visual inspection, whereas the numerical data are analyzed using both visual inspection and a more precise topological method. Contrasting the observational data with numerical data analyzed with both methods, we identify a major limitation of the visual inspection method, due to the difficulty in resolving smaller plasmoids. This result raises questions about reports of log-normal distributions of plasmoids and other coherent features in the recent literature. Based on nonlinear scaling relations of the plasmoid instability, we infer a lower bound on the current sheet width, assuming the underlying mechanism of current sheet broadening is resistive diffusion.
Note: An absolute X-Y-Θ position sensor using a two-dimensional phase-encoded binary scale
NASA Astrophysics Data System (ADS)
Kim, Jong-Ahn; Kim, Jae Wan; Kang, Chu-Shik; Jin, Jonghan
2018-04-01
This Note presents a new absolute X-Y-Θ position sensor for measuring planar motion of a precision multi-axis stage system. By analyzing the rotated image of a two-dimensional phase-encoded binary scale (2D), the absolute 2D position values at two separated points were obtained and the absolute X-Y-Θ position could be calculated combining these values. The sensor head was constructed using a board-level camera, a light-emitting diode light source, an imaging lens, and a cube beam-splitter. To obtain the uniform intensity profiles from the vignette scale image, we selected the averaging directions deliberately, and higher resolution in the angle measurement could be achieved by increasing the allowable offset size. The performance of a prototype sensor was evaluated in respect of resolution, nonlinearity, and repeatability. The sensor could resolve 25 nm linear and 0.001° angular displacements clearly, and the standard deviations were less than 18 nm when 2D grid positions were measured repeatedly.
Bidirectional Reflectance Distribution Functions For the OSIRIS-REx Target Asteroid (101955) Bennu
NASA Astrophysics Data System (ADS)
Takir, Driss; Clark, Beth E.; Lauretta, Dante S.; d'Aubigny, Christian Drouet; Hergenrother, Carl W.; Li, Jian-Yang; Binzel, Richard P.
2014-11-01
We used ground-based photometric phase curve data of asteroid (101955) Bennu and low phase-angle (proxy) data from asteroid (253) Mathilde to fit precise Modified Minnaert, Modified Lommel-Seeliger, and (RObotic Lunar Orbiter) ROLO photometric models that capture the light scattering properties of the surface and subsequently allow us to calculate the geometric albedo, phase integral, and spherical Bond albedo for this asteroid. Radiance Factor functions (RADFs) are used to model the disk-resolved brightness of Bennu. Our geometric albedo values of 0.047 ,0.047, and 0.048 for the Modified Minnaert, Modified Lommel-Seeliger, and ROLO models, respectively, are consistent with the geometric albedo of 0.030-0.045 computed by Hergenrother et al. (2013), using IAU H-G photometric system. Also, our spherical Bond albedo values of 0.016, 0.015, and 0.015 for the Minnaert model, Lommel-Seeliger, and ROLO models, respectively, are consistent with the value of 0.017 presented by Emery et al. (2014).
A predictive theory for elastic scattering and recoil of protons from 4He
Hupin, Guillaume; Quaglioni, Sofia; Navratil, Petr
2014-12-08
Low-energy cross sections for elastic scattering and recoil of protons from 4He nuclei (also known as α particles) are calculated directly by solving the Schrodinger equation for five nucleons interacting through accurate two- and three-nucleon forces derived within the framework of chiral effective field theory. Precise knowledge of these processes at various proton backscattering/recoil angles and energies is needed for the ion-beam analysis of numerous materials, from the surface layers of solids, to thin films, to fusion-reactor materials. Indeed, the same elastic scattering process, in two different kinematic configurations, can be used to probe the concentrations and depth profiles ofmore » either hydrogen or helium. Furthermore, we compare our results to available experimental data and show that direct calculations with modern nuclear potentials can help to resolve remaining inconsistencies among data sets and can be used to predict these cross sections when measurements are not available.« less
Excitation Mechanisms in Moderate-Energy Li+-He Collisions
NASA Astrophysics Data System (ADS)
Kita, Shigetomo; Itaya, Jun; Sawatari, Yugo; Tabata, Tadanobu; Hayashi, Takeo; Shimakura, Noriyuki; Koseki, Shiro
2018-02-01
Excitation mechanisms in Li+-He collisions were studied at laboratory collision energies of 350 ≤ Elab ≤ 2000 eV by measuring double differential cross sections (DCSs) σ(Θ)k over a wide range of center-of-mass scattering angles, 2.5 ≤ Θ ≤ 175°. At Elab ≥ 500 eV, two-electron (2e) excitations were observed as well as one-electron (1e) excitations. At the higher collision energies, excitation probabilities P(Θ)k for the 1e and 2e excitations have characteristic angular dependences, i.e., at Elab = 1500 and 2000 eV, P(Θ)1e for the 1e excitations has double maxima around Θ = 20 and 120° and P(Θ)2e for the 2e excitations has a broad maximum around Θ = 60°. As a first analysis of the experimental data, P(Θ)k, σ(Θ)k, and the integral cross sections Sk(Elab) were calculated by assuming excitations from the 11Σ state into the 11Π and 11Δ states through rotational couplings using the model potentials and couplings. As the next step, ab initio potential energies for the ground and excited states were calculated by a multiconfiguration self-consistent field (MCSCF) method, and then the electronic transitions among the seven states through the radial and rotational couplings were calculated using the theoretical potentials and couplings. Autoionizations from the 2e-excited He**(2s2 and 2p2) atoms were also simulated at Elab = 750-1500 eV and small laboratory angles of θ ≤ 25° by using the MCSCF potentials. The excitation mechanisms were reasonably well understood through these analyses.
An Emprical Point Error Model for Tls Derived Point Clouds
NASA Astrophysics Data System (ADS)
Ozendi, Mustafa; Akca, Devrim; Topan, Hüseyin
2016-06-01
The random error pattern of point clouds has significant effect on the quality of final 3D model. The magnitude and distribution of random errors should be modelled numerically. This work aims at developing such an anisotropic point error model, specifically for the terrestrial laser scanner (TLS) acquired 3D point clouds. A priori precisions of basic TLS observations, which are the range, horizontal angle and vertical angle, are determined by predefined and practical measurement configurations, performed at real-world test environments. A priori precision of horizontal (𝜎𝜃) and vertical (𝜎𝛼) angles are constant for each point of a data set, and can directly be determined through the repetitive scanning of the same environment. In our practical tests, precisions of the horizontal and vertical angles were found as 𝜎𝜃=±36.6𝑐𝑐 and 𝜎𝛼=±17.8𝑐𝑐, respectively. On the other hand, a priori precision of the range observation (𝜎𝜌) is assumed to be a function of range, incidence angle of the incoming laser ray, and reflectivity of object surface. Hence, it is a variable, and computed for each point individually by employing an empirically developed formula varying as 𝜎𝜌=±2-12 𝑚𝑚 for a FARO Focus X330 laser scanner. This procedure was followed by the computation of error ellipsoids of each point using the law of variance-covariance propagation. The direction and size of the error ellipsoids were computed by the principal components transformation. The usability and feasibility of the model was investigated in real world scenarios. These investigations validated the suitability and practicality of the proposed method.
NASA Astrophysics Data System (ADS)
Maeda, M.; Yamamoto, K.; Mizokawa, T.; Saini, N. L.; Arita, M.; Namatame, H.; Taniguchi, M.; Tan, G.; Zhao, L. D.; Kanatzidis, M. G.
2018-03-01
We have studied the electronic structure of SnSe and Na-doped SnSe by means of angle-resolved photoemission spectroscopy. The valence-band top reaches the Fermi level by the Na doping, indicating that Na-doped SnSe can be viewed as a degenerate semiconductor. However, in the Na-doped system, the chemical potential shift with temperature is unexpectedly large and is apparently inconsistent with the degenerate semiconductor picture. The large chemical potential shift and anomalous spectral shape are key ingredients for an understanding of the novel metallic state with the large thermoelectric performance in Na-doped SnSe.
Angle-resolved photoelectron spectroscopy of formaldehyde and methanol
NASA Astrophysics Data System (ADS)
Keller, P. R.; Taylor, J. W.; Grimm, F. A.; Carlson, Thomas A.
1984-10-01
Angle-resolved photoelectron spectroscopy was employed to obtain the angular distribution parameter, β, for the valence orbitals (IP < 21.1 eV) of formaldehyde and methanol over the 10-30 eV photon energy range using dispersed polarized synchrotron radiation as the excitation source. It was found that the energy dependence of β in the photoelectron energy range between 2 and 10 eV can be related to the molecular-orbital type from which ionization occurs. This generalized energy behavior is discussed with regard to earlier energy-dependence studies on molecules of different orbital character. Evidence is presented for the presence of resonance photoionization phenomena in formaldehyde in agreement with theoretical cross-section calculations.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Maeda, M.; Yamamoto, K.; Mizokawa, T.
In this work, we have studied the electronic structure of SnSe and Na-doped SnSe by means of angle-resolved photoemission spectroscopy. The valence-band top reaches the Fermi level by the Na doping, indicating that Na-doped SnSe can be viewed as a degenerate semiconductor. However, in the Na-doped system, the chemical potential shift with temperature is unexpectedly large and is apparently inconsistent with the degenerate semiconductor picture. Lastly, the large chemical potential shift and anomalous spectral shape are key ingredients for an understanding of the novel metallic state with the large thermoelectric performance in Na-doped SnSe.
NASA Astrophysics Data System (ADS)
van Roekeghem, Ambroise; Richard, Pierre; Shi, Xun; Wu, Shangfei; Zeng, Lingkun; Saparov, Bayrammurad; Ohtsubo, Yoshiyuki; Qian, Tian; Sefat, Athena S.; Biermann, Silke; Ding, Hong
2016-06-01
We present a study of the tetragonal to collapsed-tetragonal transition of CaFe2As2 using angle-resolved photoemission spectroscopy and dynamical mean field theory-based electronic structure calculations. We observe that the collapsed-tetragonal phase exhibits reduced correlations and a higher coherence temperature due to the stronger Fe-As hybridization. Furthermore, a comparison of measured photoemission spectra and theoretical spectral functions shows that momentum-dependent corrections to the density functional band structure are essential for the description of low-energy quasiparticle dispersions. We introduce those using the recently proposed combined "screened exchange + dynamical mean field theory" scheme.
Maeda, M.; Yamamoto, K.; Mizokawa, T.; ...
2018-03-23
In this work, we have studied the electronic structure of SnSe and Na-doped SnSe by means of angle-resolved photoemission spectroscopy. The valence-band top reaches the Fermi level by the Na doping, indicating that Na-doped SnSe can be viewed as a degenerate semiconductor. However, in the Na-doped system, the chemical potential shift with temperature is unexpectedly large and is apparently inconsistent with the degenerate semiconductor picture. Lastly, the large chemical potential shift and anomalous spectral shape are key ingredients for an understanding of the novel metallic state with the large thermoelectric performance in Na-doped SnSe.
Geometry Calibration of the SVT in the CLAS12 Detector
NASA Astrophysics Data System (ADS)
Davies, Peter; Gilfoyle, Gerard
2016-09-01
A new detector called CLAS12 is being built in Hall B as part of the 12 GeV Upgrade at Jefferson Lab to learn how quarks and gluons form nuclei. The Silicon Vertex Tracker (SVT) is one of the subsystems designed to track the trajectory of charged particles as they are emitted from the target at large angles. The sensors of the SVT consist of long, narrow, strips embedded in a silicon substrate. There are 256 strips in a sensor, with a stereo angle of 0 -3° degrees. The location of the strips must be known to a precision of a few microns in order to accurately reconstruct particle tracks with the required resolution of 50-60 microns. Our first step toward achieving this resolution was to validate the nominal geometry relative to the design specification. We also resolved differences between the design and the CLAS12, Geant4-based simulation code GEMC. We developed software to apply alignment shifts to the nominal design geometry from a survey of fiducial points on the structure that supports each sensor. The final geometry will be generated by a common package written in JAVA to ensure consistency between the simulation and Reconstruction codes. The code will be tested by studying the impact of known distortions of the nominal geometry in simulation. Work supported by the Univeristy of Richmond and the US Department of Energy.
Absolute irradiance of the Moon for on-orbit calibration
Stone, T.C.; Kieffer, H.H.; ,
2002-01-01
The recognized need for on-orbit calibration of remote sensing imaging instruments drives the ROLO project effort to characterize the Moon for use as an absolute radiance source. For over 5 years the ground-based ROLO telescopes have acquired spatially-resolved lunar images in 23 VNIR (Moon diameter ???500 pixels) and 9 SWIR (???250 pixels) passbands at phase angles within ??90 degrees. A numerical model for lunar irradiance has been developed which fits hundreds of ROLO images in each band, corrected for atmospheric extinction and calibrated to absolute radiance, then integrated to irradiance. The band-coupled extinction algorithm uses absorption spectra of several gases and aerosols derived from MODTRAN to fit time-dependent component abundances to nightly observations of standard stars. The absolute radiance scale is based upon independent telescopic measurements of the star Vega. The fitting process yields uncertainties in lunar relative irradiance over small ranges of phase angle and the full range of lunar libration well under 0.5%. A larger source of uncertainty enters in the absolute solar spectral irradiance, especially in the SWIR, where solar models disagree by up to 6%. Results of ROLO model direct comparisons to spacecraft observations demonstrate the ability of the technique to track sensor responsivity drifts to sub-percent precision. Intercomparisons among instruments provide key insights into both calibration issues and the absolute scale for lunar irradiance.
Resonances in the Field-Angle-Resolved Thermal Conductivity of CeCoIn 5
Kim, Duk Y.; Lin, Shi -Zeng; Weickert, Franziska; ...
2017-05-12
Here, the thermal conductivity measurement in a rotating magnetic field is a powerful probe of the structure of the superconducting energy gap. We present high-precision measurements of the low-temperature thermal conductivity in the unconventional heavy-fermion superconductor CeCoIn 5, with the heat current J along the nodal [110] direction of its d x2–y2 order parameter and the magnetic field up to 7 T rotating in the ab plane. In contrast to the smooth oscillations found previously for J∥[100], we observe a sharp resonancelike peak in the thermal conductivity when the magnetic field is also in the [110] direction, parallel to themore » heat current. We explain this peak qualitatively via a model of the heat transport in a d-wave superconductor. In addition, we observe two smaller but also very sharp peaks in the thermal conductivity for the field directions at angles Θ≈±33° with respect to J. The origin of the observed resonances at Θ≈±33° at present defies theoretical explanation. The challenge of uncovering their source will dictate exploring theoretically more complex models, which might include, e.g., fine details of the Fermi surface, Andreev bound vortex core states, a secondary superconducting order parameter, and the existence of gaps in spin and charge excitations.« less
Resonances in the Field-Angle-Resolved Thermal Conductivity of CeCoIn 5
DOE Office of Scientific and Technical Information (OSTI.GOV)
Kim, Duk Y.; Lin, Shi -Zeng; Weickert, Franziska
Here, the thermal conductivity measurement in a rotating magnetic field is a powerful probe of the structure of the superconducting energy gap. We present high-precision measurements of the low-temperature thermal conductivity in the unconventional heavy-fermion superconductor CeCoIn 5, with the heat current J along the nodal [110] direction of its d x2–y2 order parameter and the magnetic field up to 7 T rotating in the ab plane. In contrast to the smooth oscillations found previously for J∥[100], we observe a sharp resonancelike peak in the thermal conductivity when the magnetic field is also in the [110] direction, parallel to themore » heat current. We explain this peak qualitatively via a model of the heat transport in a d-wave superconductor. In addition, we observe two smaller but also very sharp peaks in the thermal conductivity for the field directions at angles Θ≈±33° with respect to J. The origin of the observed resonances at Θ≈±33° at present defies theoretical explanation. The challenge of uncovering their source will dictate exploring theoretically more complex models, which might include, e.g., fine details of the Fermi surface, Andreev bound vortex core states, a secondary superconducting order parameter, and the existence of gaps in spin and charge excitations.« less
Peripapillary schisis in open-angle glaucoma.
Dhingra, N; Manoharan, R; Gill, S; Nagar, M
2017-03-01
PurposeTo report clinical features, topographic findings and outcome of 10 eyes with peripapillary schisis in open-angle glaucoma.Patients and methodsA retrospective review of patients with open-angle glaucoma who were noted to have peripapillary schisis on optical coherence tomography (OCT) were included. Serial peripapillary and macula infrared and OCT images, visual acuity, visual fields, and schisis appearance were reviewed.ResultsTen eyes of nine patients with open-angle glaucoma were detected to have the presence of peripapillary schisis. Nerve fibre layer schisis was detected in all eyes and one eye had an associated macular schisis. None of the eyes had an acquired pit of the optic nerve or pathological myopia. The mean intraocular pressures at detection was 18.3±4.3 mm Hg and the schisis resolved in four eyes after a mean follow-up of 21.2±8.8 months. Visual field worsening was noted in 4 of the 10 eyes and the resolution of schisis resulted in significant reduction in the retinal nerve fibre layer (RNFL) thickness.ConclusionsPeripapillary schisis detected during the normal course of open-angle glaucoma can resolve spontaneously and rarely involves the macula. Its resolution leads to reduction in RNFL thickness; therefore, caution is advised while interpreting serial scans.
Materials characterisation by angle-resolved scanning transmission electron microscopy.
Müller-Caspary, Knut; Oppermann, Oliver; Grieb, Tim; Krause, Florian F; Rosenauer, Andreas; Schowalter, Marco; Mehrtens, Thorsten; Beyer, Andreas; Volz, Kerstin; Potapov, Pavel
2016-11-16
Solid-state properties such as strain or chemical composition often leave characteristic fingerprints in the angular dependence of electron scattering. Scanning transmission electron microscopy (STEM) is dedicated to probe scattered intensity with atomic resolution, but it drastically lacks angular resolution. Here we report both a setup to exploit the explicit angular dependence of scattered intensity and applications of angle-resolved STEM to semiconductor nanostructures. Our method is applied to measure nitrogen content and specimen thickness in a GaN x As 1-x layer independently at atomic resolution by evaluating two dedicated angular intervals. We demonstrate contrast formation due to strain and composition in a Si- based metal-oxide semiconductor field effect transistor (MOSFET) with Ge x Si 1-x stressors as a function of the angles used for imaging. To shed light on the validity of current theoretical approaches this data is compared with theory, namely the Rutherford approach and contemporary multislice simulations. Inconsistency is found for the Rutherford model in the whole angular range of 16-255 mrad. Contrary, the multislice simulations are applicable for angles larger than 35 mrad whereas a significant mismatch is observed at lower angles. This limitation of established simulations is discussed particularly on the basis of inelastic scattering.
Modified sine bar device measures small angles with high accuracy
NASA Technical Reports Server (NTRS)
Thekaekara, M.
1968-01-01
Modified sine bar device measures small angles with enough accuracy to calibrate precision optical autocollimators. The sine bar is a massive bar of steel supported by two cylindrical rods at one end and one at the other.
NASA Astrophysics Data System (ADS)
Jouybari, A.; Ardalan, A. A.; Rezvani, M.-H.
2017-09-01
The accurate measurement of platform orientation plays a critical role in a range of applications including marine, aerospace, robotics, navigation, human motion analysis, and machine interaction. We used Mahoney filter, Complementary filter and Xsens Kalman filter for achieving Euler angle of a dynamic platform by integration of gyroscope, accelerometer, and magnetometer measurements. The field test has been performed in Kish Island using an IMU sensor (Xsens MTi-G-700) that installed onboard a buoy so as to provide raw data of gyroscopes, accelerometers, magnetometer measurements about 25 minutes. These raw data were used to calculate the Euler angles by Mahoney filter and Complementary filter, while the Euler angles collected by XSense IMU sensor become the reference of the Euler angle estimations. We then compared Euler angles which calculated by Mahoney Filter and Complementary Filter with reference to the Euler angles recorded by the XSense IMU sensor. The standard deviations of the differences between the Mahoney Filter, Complementary Filter Euler angles and XSense IMU sensor Euler angles were about 0.5644, 0.3872, 0.4990 degrees and 0.6349, 0.2621, 2.3778 degrees for roll, pitch, and heading, respectively, so the numerical result assert that Mahoney filter is precise for roll and heading angles determination and Complementary filter is precise only for pitch determination, it should be noted that heading angle determination by Complementary filter has more error than Mahoney filter.
NASA Astrophysics Data System (ADS)
Ye, Dong; Sun, Zhaowei; Wu, Shunan
2012-08-01
The quaternion-based, high precision, large angle rapid reorientation of rigid spacecraft is the main problem investigated in this study. The operation is accomplished via a hybrid thrusters and reaction wheels strategy where thrusters are engaged in providing a primary maneuver torque in open loop, while reaction wheels provide fine control torque to achieve high precision in closed-loop control. The inaccuracy of thrusters is handled by a variable structure control (VSC). In addition, a signum function is mixed in the switching surface in VSC to produce a maneuver to the reference attitude trajectory in a shortest distance. Detailed proofs and numerical simulation examples are presented to illustrate all the technical aspects of this work.
NASA Astrophysics Data System (ADS)
Lyo, In-Whan
Electronic properties of the epitaxially grown Na(110) film have been studied using angle resolved ultraviolet photoemission spectroscopy with synchrotron radiation as the light source. Na provides an ideal ground to study the fundamental aspects of the electron-electron interactions in metals, because of its simple Fermi surface and small pseudopotential. The absolute band structure of Na(110) using angle resolved photoemission spectroscopy has been mapped out using the extrema searching method. The advantage of this approach is that the usual assumption of the unoccupied state dispersion is not required. We have found that the dispersion of Na(1l0) is very close to the parabolic band with the effective mass 1.21 M_{rm e} at 90 K. Self-consistent calculations of the self-energy for the homogeneous electron gas have been performed using the Green's function technique within the framework of the GW approximation, in the hope of understanding the narrowing mechanism of the bandwidth observed for all the nearly-free-electron (NFE) metals. Good agreements between the experimental data and our calculated self-energy were obtained not only for our data on k-dependency from Na(l10), but also for the total bandwidth corrections for other NFE metals, only if dielectric functions beyond the random phase approximation were used. Our findings emphasize the importance of the screening by long wavelength plasmons. Off-normal spectra of angle resolved photoemission from Na(110) show strong asymmetry of the bulk peak intensity for the wide range of photon energies. Using a simple analysis, we show this asymmetry has an origin in the interference of the surface Umklapp electrons with the normal electrons. We have also performed the detailed experimental studies of the anomalous Fermi level structure observed in the forbidden gap region of Na. This was claimed by A. W. Overhauser as the evidence of the charge density wave in the alkali metal. The possibility of this hypothesis is critically discussed against other explanations.
Ramsey-type spectroscopy in the XUV spectral region
DOE Office of Scientific and Technical Information (OSTI.GOV)
Pirri, A.; European Laboratory for Nonlinear Spectroscopy, Via N. Carrara 1, I-50019 Sesto Fiorentino; Sali, E.
2010-02-02
We report an experimental and theoretical investigation of Ramsey-type spectroscopy with high-order harmonic generation applied to autoionizing states of Krypton. The ionization yield, detected by an ion-mass spectrometer, shows the characteristic quantum interference pattern. The behaviour of the fringe contrast was interpreted on the basis of a simple analytic model, which reproduces the experimental data without any free parameter.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Hahn, M.; Novotny, O.; Savin, D. W.
2013-04-10
We report measurements of electron impact ionization for Fe{sup 13+}, Fe{sup 16+}, and Fe{sup 17+} over collision energies from below threshold to above 3000 eV. The ions were recirculated using an ion storage ring. Data were collected after a sufficiently long time that essentially all the ions had relaxed radiatively to their ground state. For single ionization of Fe{sup 13+}, we find that previous single pass experiments are more than 40% larger than our results. Compared to our work, the theoretical cross section recommended by Arnaud and Raymond is more than 30% larger, while that of Dere is about 20%more » greater. Much of the discrepancy with Dere is due to the theory overestimating the contribution of excitation-autoionization via n = 2 excitations. Double ionization of Fe{sup 13+} is dominated by direct ionization of an inner shell electron accompanied by autoionization of a second electron. Our results for single ionization of Fe{sup 16+} and Fe{sup 17+} agree with theoretical calculations to within the experimental uncertainties.« less
Quasiclassical treatment of the Auger effect in slow ion-atom collisions
NASA Astrophysics Data System (ADS)
Frémont, F.
2017-09-01
A quasiclassical model based on the resolution of Hamilton equations of motion is used to get evidence for Auger electron emission following double-electron capture in 150-keV N e10 ++He collisions. Electron-electron interaction is taken into account during the collision by using pure Coulombic potential. To make sure that the helium target is stable before the collision, phenomenological potentials for the electron-nucleus interactions that simulate the Heisenberg principle are included in addition to the Coulombic potential. First, single- and double-electron captures are determined and compared with previous experiments and theories. Then, integration time evolution is calculated for autoionizing and nonautoionizing double capture. In contrast with single capture, the number of electrons originating from autoionization slowly increases with integration time. A fit of the calculated cross sections by means of an exponential function indicates that the average lifetime is 4.4 ×10-3a .u . , in very good agreement with the average lifetime deduced from experiments and a classical model introduced to calculate individual angular momentum distributions. The present calculation demonstrates the ability of classical models to treat the Auger effect, which is a pure quantum effect.
Electron-impact ionization of P-like ions forming Si-like ions
DOE Office of Scientific and Technical Information (OSTI.GOV)
Kwon, D.-H.; Savin, D. W., E-mail: hkwon@kaeri.re.kr
2014-03-20
We have calculated electron-impact ionization (EII) for P-like systems from P to Zn{sup 15+} forming Si-like ions. The work was performed using the flexible atomic code (FAC) which is based on a distorted-wave approximation. All 3ℓ → nℓ' (n = 3-35) excitation-autoionization (EA) channels near the 3p direct ionization threshold and 2ℓ → nℓ' (n = 3-10) EA channels at the higher energies are included. Close attention has been paid to the detailed branching ratios. Our calculated total EII cross sections are compared both with previous FAC calculations, which omitted many of these EA channels, and with the available experimentalmore » results. Moreover, for Fe{sup 11+}, we find that part of the remaining discrepancies between our calculations and recent measurements can be accounted for by the inclusion of the resonant excitation double autoionization process. Lastly, at the temperatures where each ion is predicted to peak in abundances in collisional ionization equilibrium, the Maxwellian rate coefficients derived from our calculations differ by 50%-7% from the previous FAC rate coefficients, with the difference decreasing with increasing charge.« less
Shen, Bing; Yu, Li; Liu, Kai; ...
2017-06-01
We have carried out high-resolution angle-resolved photoemission measurements on the Cebased heavy fermion compound CePt 2In 7 that exhibits stronger two-dimensional character than the prototypical heavy fermion system CeCoIn 5. Multiple Fermi surface sheets and a complex band structure are clearly resolved. We have also performed detailed band structure calculations on CePt 2In 7. The good agreement found between our measurements and the calculations suggests that the band renormalization effect is rather weak in CePt 2In 7. A comparison of the common features of the electronic structure of CePt 2In 7 and CeCoIn5 indicates that CeCoIn 5 shows a muchmore » stronger band renormalization effect than CePt 2In 7. These results provide new information for understanding the heavy fermion behaviors and unconventional superconductivity in Ce-based heavy fermion systems.« less
Liu, Ro-Ya; Ogawa, Yu; Chen, Peng; Ozawa, Kenichi; Suzuki, Takeshi; Okada, Masaru; Someya, Takashi; Ishida, Yukiaki; Okazaki, Kozo; Shin, Shik; Chiang, Tai-Chang; Matsuda, Iwao
2017-11-22
Time-dependent responses of materials to an ultrashort optical pulse carry valuable information about the electronic and lattice dynamics; this research area has been widely studied on novel two-dimensional materials such as graphene, transition metal dichalcogenides (TMDs) and topological insulators (TIs). We report herein a time-resolved and angle-resolved photoemission spectroscopy (TRARPES) study of WSe 2 , a layered semiconductor of interest for valley electronics. The results for below-gap optical pumping reveal energy-gain and -loss Floquet replica valence bands that appear instantaneously in concert with the pump pulse. Energy shift, broadening, and complex intensity variation and oscillation at twice the phonon frequency for the valence bands are observed at time scales ranging from the femtosecond to the picosecond and beyond. The underlying physics is rich, including ponderomotive interaction, dressing of the electronic states, creation of coherent phonon pairs, and diffusion of charge carriers - effects operating at vastly different time domains.
Analysis of Massively Separated Flows of Aircraft Using Detached Eddy Simulation
NASA Astrophysics Data System (ADS)
Morton, Scott
2002-08-01
An important class of turbulent flows of aerodynamic interest are those characterized by massive separation, e.g., the flow around an aircraft at high angle of attack. Numerical simulation is an important tool for analysis, though traditional models used in the solution of the Reynolds-averaged Navier-Stokes (RANS) equations appear unable to accurately account for the time-dependent and three-dimensional motions governing flows with massive separation. Large-eddy simulation (LES) is able to resolve these unsteady three-dimensional motions, yet is cost prohibitive for high Reynolds number wall-bounded flows due to the need to resolve the small scale motions in the boundary layer. Spalart et. al. proposed a hybrid technique, Detached-Eddy Simulation (DES), which takes advantage of the often adequate performance of RANS turbulence models in the "thin," typically attached regions of the flow. In the separated regions of the flow the technique becomes a Large Eddy Simulation, directly resolving the time-dependent and unsteady features that dominate regions of massive separation. The current work applies DES to a 70 degree sweep delta wing at 27 degrees angle of attack, a geometrically simple yet challenging flowfield that exhibits the unsteady three-dimensional massively separated phenomena of vortex breakdown. After detailed examination of this basic flowfield, the method is demonstrated on three full aircraft of interest characterized by massive separation, the F-16 at 45 degrees angle of attack, the F-15 at 65 degree angle of attack (with comparison to flight test), and the C-130 in a parachute drop condition at near stall speed with cargo doors open.
Angle classification revisited 2: a modified Angle classification.
Katz, M I
1992-09-01
Edward Angle, in his classification of malocclusions, appears to have made Class I a range of abnormality, not a point of ideal occlusion. Current goals of orthodontic treatment, however, strive for the designation "Class I occlusion" to be synonymous with the point of ideal intermeshing and not a broad range. If contemporary orthodontists are to continue to use Class I as a goal, then it is appropriate that Dr. Angle's century-old classification, be modified to be more precise.
Selectively enhanced photocurrent generation in twisted bilayer graphene with van Hove singularity
Yin, Jianbo; Wang, Huan; Peng, Han; Tan, Zhenjun; Liao, Lei; Lin, Li; Sun, Xiao; Koh, Ai Leen; Chen, Yulin; Peng, Hailin; Liu, Zhongfan
2016-01-01
Graphene with ultra-high carrier mobility and ultra-short photoresponse time has shown remarkable potential in ultrafast photodetection. However, the broad and weak optical absorption (∼2.3%) of monolayer graphene hinders its practical application in photodetectors with high responsivity and selectivity. Here we demonstrate that twisted bilayer graphene, a stack of two graphene monolayers with an interlayer twist angle, exhibits a strong light–matter interaction and selectively enhanced photocurrent generation. Such enhancement is attributed to the emergence of unique twist-angle-dependent van Hove singularities, which are directly revealed by spatially resolved angle-resolved photoemission spectroscopy. When the energy interval between the van Hove singularities of the conduction and valance bands matches the energy of incident photons, the photocurrent generated can be significantly enhanced (up to ∼80 times with the integration of plasmonic structures in our devices). These results provide valuable insight for designing graphene photodetectors with enhanced sensitivity for variable wavelength. PMID:26948537
DOE Office of Scientific and Technical Information (OSTI.GOV)
He, Junfeng; Mion, Thomas R.; Gao, Shang
2016-10-31
Unraveling the nature of pseudogap phase in high-temperature superconductors holds the key to understanding their superconducting mechanisms and potentially broadening their applications via enhancement of their superconducting transition temperatures. Angle-resolved photoemission spectroscopy (ARPES) experiments using circularly polarized light have been proposed to detect possible symmetry breaking state in the pseudogap phase of cuprates. Here, the presence (absence) of an electronic order which breaks mirror symmetry of the crystal would in principle induce a finite (zero) circular dichroism in photoemission. Different orders breaking reflection symmetries about different mirror planes can also be distinguished by the momentum dependence of the measured circularmore » dichroism.« less
Zhu, Yizheng; Terry, Neil G; Wax, Adam
2012-01-01
Angle-resolved low-coherence interferometry (a/LCI) is an optical biopsy technique that measures scattered light from tissue to determine nuclear size with submicron-level accuracy. The a/LCI probe can be deployed through the accessory channel of a standard endoscope and provides feedback to physicians to guide physical biopsies. The technique has been validated in animal and ex vivo human studies, and has been used to detect dysplasia in Barrett’s esophagus patients in vivo. In a recent clinical study of 46 Barrett’s esophagus patients, a/LCI was able to detect dysplasia with 100% sensitivity and 84% specificity. This report reviews the technique and discusses its potential clinical utility. PMID:22149580
Destroying coherence in high-temperature superconductors with current flow
Kaminski, A.; Rosenkranz, S.; Norman, M. R.; ...
2016-09-13
Here, the loss of single-particle coherence going from the superconducting state to the normal state in underdoped cuprates is a dramatic effect that has yet to be understood. Here, we address this issue by performing angle resolved photoemission spectroscopy measurements in the presence of a transport current. We find that the loss of coherence is associated with the development of an onset in the resistance, in that well before the midpoint of the transition is reached, the sharp peaks in the angle resolved photoemission spectra are completely suppressed. Since the resistance onset is a signature of phase fluctuations, this impliesmore » that the loss of single-particle coherence is connected with the loss of long-range phase coherence.« less
NASA Astrophysics Data System (ADS)
Sun, Yue; Kittaka, Shunichiro; Nakamura, Shota; Sakakibara, Toshiro; Irie, Koki; Nomoto, Takuya; Machida, Kazushige; Chen, Jingting; Tamegai, Tsuyoshi
2017-12-01
Quasiparticle excitations in FeSe were studied by means of specific heat (C ) measurements on a high-quality single crystal under rotating magnetic fields. The field dependence of C shows three-stage behavior with different slopes, indicating the existence of three gaps (Δ1,Δ2, and Δ3). In the low-temperature and low-field region, the azimuthal angle (ϕ ) dependence of C shows a fourfold symmetric oscillation with a sign change. On the other hand, the polar angle (θ ) dependence manifests as an anisotropy-inverted twofold symmetry with unusual shoulder behavior. Combining the angle-resolved results and the theoretical calculation, the smaller gap Δ1 is proved to have two vertical-line nodes or gap minima along the kz direction, and is determined to reside on the electron-type ɛ band. Δ2 is found to be related to the electron-type δ band, and is isotropic in the a b plane but largely anisotropic out of the plane. Δ3 residing on the hole-type α band shows a small out-of-plane anisotropy with a strong Pauli paramagnetic effect.
Self-Assembly of Hierarchical DNA Nanotube Architectures with Well-Defined Geometries.
Jorgenson, Tyler D; Mohammed, Abdul M; Agrawal, Deepak K; Schulman, Rebecca
2017-02-28
An essential motif for the assembly of biological materials such as actin at the scale of hundreds of nanometers and beyond is a network of one-dimensional fibers with well-defined geometry. Here, we demonstrate the programmed organization of DNA filaments into micron-scale architectures where component filaments are oriented at preprogrammed angles. We assemble L-, T-, and Y-shaped DNA origami junctions that nucleate two or three micron length DNA nanotubes at high yields. The angles between the nanotubes mirror the angles between the templates on the junctions, demonstrating that nanoscale structures can control precisely how micron-scale architectures form. The ability to precisely program filament orientation could allow the assembly of complex filament architectures in two and three dimensions, including circuit structures, bundles, and extended materials.
Bull, James N.; West, Christopher W.
2015-01-01
Frequency-, angle-, and time-resolved photoelectron imaging of gas-phase menadione (vitamin K3) radical anions was used to show that quasi-bound resonances of the anion can act as efficient doorway states to produce metastable ground electronic state anions on a sub-picosecond timescale. Several anion resonances have been experimentally observed and identified with the assistance of ab initio calculations, and ground state anion recovery was observed across the first 3 eV above threshold. Time-resolved measurements revealed the mechanism of electronic ground state anion formation, which first involves a cascade of very fast internal conversion processes to a bound electronic state that, in turn, decays by slower internal conversion to the ground state. Autodetachment processes from populated resonances are inefficient compared with electronic relaxation through internal conversion. The mechanistic understanding gained provides insight into the formation of radical anions in biological and astrochemical systems. PMID:29560245
Eliminating Deadbands In Resistive Angle Sensors
NASA Technical Reports Server (NTRS)
Salomon, Phil M.; Allen, Russell O.; Marchetto, Carl A.
1992-01-01
Proposed shaft-angle-measuring circuit provides continuous indication of angle of rotation from 0 degree to 360 degrees. Sensing elements are two continuous-rotation potentiometers, and associated circuitry eliminates deadband that occurs when wiper contact of potentiometer crosses end contacts near 0 degree position of circular resistive element. Used in valve-position indicator or similar device in which long operating life and high angular precision not required.
ERIC Educational Resources Information Center
Bindel, Thomas H.
2010-01-01
Entropy analyses as a function of the extent of reaction are presented for a number of physicochemical processes, including vaporization of a liquid, dimerization of nitrogen dioxide, and the autoionization of water. Graphs of the total entropy change versus the extent of reaction give a visual representation of chemical equilibrium and the second…
Electronic Structure of Helium Atom in a Quantum Dot
NASA Astrophysics Data System (ADS)
Saha, Jayanta K.; Bhattacharyya, S.; Mukherjee, T. K.
2016-03-01
Bound and resonance states of helium atom have been investigated inside a quantum dot by using explicitly correlated Hylleraas type basis set within the framework of stabilization method. To be specific, precise energy eigenvalues of bound 1sns (1Se) (n = 1-6) states and the resonance parameters i.e. positions and widths of 1Se states due to 2sns (n = 2-5) and 2pnp (n = 2-5) configurations of confined helium below N = 2 ionization threshold of He+ have been estimated. The two-parameter (Depth and Width) finite oscillator potential is used to represent the confining potential due to the quantum dot. It has been explicitly demonstrated that the electronic structural properties become sensitive functions of the dot size. It is observed from the calculations of ionization potential that the stability of an impurity ion within a quantum dot may be manipulated by varying the confinement parameters. A possibility of controlling the autoionization lifetime of doubly excited states of two-electron ions by tuning the width of the quantum cavity is also discussed here. TKM Gratefully Acknowledges Financial Support under Grant No. 37(3)/14/27/2014-BRNS from the Department of Atomic Energy, BRNS, Government of India. SB Acknowledges Financial Support under Grant No. PSW-160/14-15(ERO) from University Grants Commission, Government of India
NASA Astrophysics Data System (ADS)
Haque, Ghousia Nasreen
The absorption of electromagnetic radiation by positive ions is one of the fundamental processes of nature which occurs in every intensely hot environment. Due to the difficulties in producing sufficient densities of ions in a laboratory, there are very few measurements of ionic photoabsorption parameters. On the theoretical side, some calculations have been made of a few major photoionization parameters, but generally speaking, most of the work done so far has employed rather simple single particle models and any theoretical work which has adequately taken into account intricate atomic many-body and relativistic effects is only scanty. In the present work, several complex aspects of atomic/ionic photoabsorption parameters have been studied. Non -resonant photoionization in neon and argon isonuclear as well as isoelectronic sequences has been studied using a very sophisticated technique, namely the relativistic random phase approximation (RRPA). This technique takes into account relativistic effects as well as an important class of major many-body effects on the same footing. The present calculations confirmed that gross features of photoionization parameters calculated using simpler models were not an artifact of the simple model. Also, the present RRPA calculations on K^+ ion and neutral Ar brought out the relative importance of various many-body effects such the inter-channel coupling. Inter-channel coupling between discrete bound state photoexcitation channels from an inner atomic/ionic level and photoionization continuum channels from an outer atomic/ionic level leads to the phenomena of autoionization resonances in the photoionization process. These resonances lead to very complex effects in the atomic/ionic photoabsorption spectra. These resonances have been calculated and studied in the present work in the neon and magnesium isoelectronic sequences using the relativistic multi-channel quantum defect theory (RMQDT) within the framework of the RRPA. The character of the autoionization resonances studied was determined in the present work and the effect of series perturbations in the Rydberg series due to interference between various multichannel processes was quantitatively determined. Furthermore, results of the present calculations also serve as important pointer to measure the relative strengths of radiative (fluorescence) decay modes and non -radiative (autoionization/auger) decay modes in an isoelectronic sequence.
Flare angles measured with ball gage
NASA Technical Reports Server (NTRS)
Cleghorn, D.; Wall, W. A.
1968-01-01
Precision tungsten carbide balls measure the internal angle of flared joints. Measurements from small and large balls in the flare throat to an external reference point are made. The difference in distances and diameters determine the average slope of the flare between the points of ball contact.
Flight Performance of a Man Portable Guided Projectile Concept
2014-02-01
include precision guided technologies. The focus of this study is maneuvering projectiles launched from man portable weapon systems . A novel guided...5 Figure 5. Body-fixed coordinate system and aerodynamic angles...20 Figure 20. Earth and body-fixed coordinate systems and Euler angles. ........................................24
Minakata, Hisakazu; Parke, Stephen J.
2013-06-04
Precision measurement of the leptonic CP violating phase δ will suffer from the, then surviving, large uncertainty of sin 2θ 23 of 10–20% in the experimentally interesting region near maximal mixing of θ 23. We advocate a new method for determination of both θ 23 and δ at the same time using only the ν e and ν̄ e appearance channels and show that sin 2θ 23 can be determined automatically with much higher accuracy, approximately a factor of six, than sinδ. In this method, we identify a new degeneracy for the simultaneous determination of θ 23 and δ, themore » θ 23 intrinsic degeneracy, which must be resolved in order to achieve precision measurement of these two parameters. Spectral information around the vacuum oscillation maxima is shown to be the best way to resolve this degeneracy.« less
Quantifying the Precision of Single-Molecule Torque and Twist Measurements Using Allan Variance.
van Oene, Maarten M; Ha, Seungkyu; Jager, Tessa; Lee, Mina; Pedaci, Francesco; Lipfert, Jan; Dekker, Nynke H
2018-04-24
Single-molecule manipulation techniques have provided unprecedented insights into the structure, function, interactions, and mechanical properties of biological macromolecules. Recently, the single-molecule toolbox has been expanded by techniques that enable measurements of rotation and torque, such as the optical torque wrench (OTW) and several different implementations of magnetic (torque) tweezers. Although systematic analyses of the position and force precision of single-molecule techniques have attracted considerable attention, their angle and torque precision have been treated in much less detail. Here, we propose Allan deviation as a tool to systematically quantitate angle and torque precision in single-molecule measurements. We apply the Allan variance method to experimental data from our implementations of (electro)magnetic torque tweezers and an OTW and find that both approaches can achieve a torque precision better than 1 pN · nm. The OTW, capable of measuring torque on (sub)millisecond timescales, provides the best torque precision for measurement times ≲10 s, after which drift becomes a limiting factor. For longer measurement times, magnetic torque tweezers with their superior stability provide the best torque precision. Use of the Allan deviation enables critical assessments of the torque precision as a function of measurement time across different measurement modalities and provides a tool to optimize measurement protocols for a given instrument and application. Copyright © 2018 Biophysical Society. Published by Elsevier Inc. All rights reserved.
NASA Astrophysics Data System (ADS)
Sander, M.; Pudell, J.-E.; Herzog, M.; Bargheer, M.; Bauer, R.; Besse, V.; Temnov, V.; Gaal, P.
2017-12-01
We present time-resolved x-ray reflectivity measurements on laser excited coherent and incoherent surface deformations of thin metallic films. Based on a kinematical diffraction model, we derive the surface amplitude from the diffracted x-ray intensity and resolve transient surface excursions with sub-Å spatial precision and 70 ps temporal resolution. The analysis allows for decomposition of the surface amplitude into multiple coherent acoustic modes and a substantial contribution from incoherent phonons which constitute the sample heating.
Cross-sectional structural parameters from densitometry
NASA Technical Reports Server (NTRS)
Cleek, Tammy M.; Whalen, Robert T.
2002-01-01
Bone densitometry has previously been used to obtain cross-sectional properties of bone from a single X-ray projection across the bone width. Using three unique projections, we have extended the method to obtain the principal area moments of inertia and orientations of the principal axes at each scan cross-section along the length of the scan. Various aluminum phantoms were used to examine scanner characteristics to develop the highest accuracy possible for in vitro non-invasive analysis of cross-sectional properties. Factors considered included X-ray photon energy, initial scan orientation, the angle spanned by the three scans (included angle), and I(min)/I(max) ratios. Principal moments of inertia were accurate to within +/-3.1% and principal angles were within +/-1 degrees of the expected value for phantoms scanned with included angles of 60 degrees and 90 degrees at the higher X-ray photon energy (140 kVp). Low standard deviations in the error (0.68-1.84%) also indicate high precision of calculated measurements with these included angles. Accuracy and precision decreased slightly when the included angle was reduced to 30 degrees. The method was then successfully applied to a pair of excised cadaveric tibiae. The accuracy and insensitivity of the algorithms to cross-sectional shape and changing isotropy (I(min)/I(max)) values when various included angles are used make this technique viable for future in vivo studies.
Laser interferometric high-precision angle monitor for JASMINE
NASA Astrophysics Data System (ADS)
Niwa, Yoshito; Arai, Koji; Sakagami, Masaaki; Gouda, Naoteru; Kobayashi, Yukiyasu; Yamada, Yoshiyuki; Yano, Taihei
2006-06-01
The JASMINE instrument uses a beam combiner to observe two different fields of view separated by 99.5 degrees simultaneously. This angle is so-called basic angle. The basic angle of JASMINE should be stabilized and fluctuations of the basic angle should be monitored with the accuracy of 10 microarcsec in root-mean-square over the satellite revolution period of 5 hours. For this purpose, a high-precision interferometric laser metrogy system is employed. One of the available techniques for measuring the fluctuations of the basic angle is a method known as the wave front sensing using a Fabry-Perot type laser interferometer. This technique is to detect fluctuations of the basic angle as displacement of optical axis in the Fabry-Perot cavity. One of the advantages of the technique is that the sensor is made to be sensitive only to the relative fluctuations of the basic angle which the JASMINE wants to know and to be insensitive to the common one; in order to make the optical axis displacement caused by relative motion enhanced the Fabry-Perot cavity is formed by two mirrors which have long radius of curvature. To verify the principle of this idea, the experiment was performed using a 0.1m-length Fabry-Perot cavity with the mirror curvature of 20m. The mirrors of the cavity were artificially actuated in either relative way or common way and the resultant outputs from the sensor were compared.
Palmer, T. N.
2014-01-01
This paper sets out a new methodological approach to solving the equations for simulating and predicting weather and climate. In this approach, the conventionally hard boundary between the dynamical core and the sub-grid parametrizations is blurred. This approach is motivated by the relatively shallow power-law spectrum for atmospheric energy on scales of hundreds of kilometres and less. It is first argued that, because of this, the closure schemes for weather and climate simulators should be based on stochastic–dynamic systems rather than deterministic formulae. Second, as high-wavenumber elements of the dynamical core will necessarily inherit this stochasticity during time integration, it is argued that the dynamical core will be significantly over-engineered if all computations, regardless of scale, are performed completely deterministically and if all variables are represented with maximum numerical precision (in practice using double-precision floating-point numbers). As the era of exascale computing is approached, an energy- and computationally efficient approach to cloud-resolved weather and climate simulation is described where determinism and numerical precision are focused on the largest scales only. PMID:24842038
Palmer, T N
2014-06-28
This paper sets out a new methodological approach to solving the equations for simulating and predicting weather and climate. In this approach, the conventionally hard boundary between the dynamical core and the sub-grid parametrizations is blurred. This approach is motivated by the relatively shallow power-law spectrum for atmospheric energy on scales of hundreds of kilometres and less. It is first argued that, because of this, the closure schemes for weather and climate simulators should be based on stochastic-dynamic systems rather than deterministic formulae. Second, as high-wavenumber elements of the dynamical core will necessarily inherit this stochasticity during time integration, it is argued that the dynamical core will be significantly over-engineered if all computations, regardless of scale, are performed completely deterministically and if all variables are represented with maximum numerical precision (in practice using double-precision floating-point numbers). As the era of exascale computing is approached, an energy- and computationally efficient approach to cloud-resolved weather and climate simulation is described where determinism and numerical precision are focused on the largest scales only.
Three Dimensional Cross-Sectional Properties From Bone Densitometry
NASA Technical Reports Server (NTRS)
Cleek, Tammy M.; Whalen, Robert T.; Dalton, Bonnie P. (Technical Monitor)
2001-01-01
Bone densitometry has previously been used to obtain cross-sectional properties of bone in a single scan plane. Using three non-coplanar scans, we have extended the method to obtain the principal area Moments of inertia and orientations of the principal axes at each cross-section along the length of the scan. Various 5 aluminum phantoms were used to examine scanner characteristics to develop the highest accuracy possible for in vitro non-invasive analysis of mass distribution. Factors considered included X-ray photon energy, initial scan orientation, the included angle of the 3 scans, and Imin/Imax ratios. Principal moments of inertia were accurate to within 3.1% and principal angles were within 1 deg. of the expected value for phantoms scanned with included angles of 60 deg. and 90 deg. at the higher X-ray photon energy. Low standard deviations in error also 10 indicate high precision of calculated measurements with these included angles. Accuracy and precision decreased slightly when the included angle was reduced to 30 deg. The method was then successfully applied to a pair of excised cadaveric tibiae. The accuracy and insensitivity of the algorithms to cross-sectional shape and changing isotropy (Imin/Imax) values when various included angles are used make this technique viable for future in vivo studies.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Yang, Siqi
2016-01-01
We present a measurement of the fundamental parameter of the standard model, the weak mixing angle, in pp¯→Z/γ∗→e+e− events at a center of mass energy of 1.96 TeV, using data corresponding to 9.7 fb−1 of integrated luminosity collected by the D0 detector at the Fermilab Tevatron. The effective weak mixing angle is extracted from the forward-backward charge asymmetry as a function of the invariant mass around the Z boson pole. The measured value of sin2θℓeff=0.23147±0.00047 is the most precise measurement from light quark interactions to date, with a precision close to the best LEP and SLD results.
Precise determination of lattice phase shifts and mixing angles
Lu, Bing -Nan; Lähde, Timo A.; Lee, Dean; ...
2016-07-09
Here, we introduce a general and accurate method for determining lattice phase shifts and mixing angles, which is applicable to arbitrary, non-cubic lattices. Our method combines angular momentum projection, spherical wall boundaries and an adjustable auxiliary potential. This allows us to construct radial lattice wave functions and to determine phase shifts at arbitrary energies. For coupled partial waves, we use a complex-valued auxiliary potential that breaks time-reversal invariance. We benchmark our method using a system of two spin-1/2 particles interacting through a finite-range potential with a strong tensor component. We are able to extract phase shifts and mixing angles formore » all angular momenta and energies, with precision greater than that of extant methods. We discuss a wide range of applications from nuclear lattice simulations to optical lattice experiments.« less
Research on Precision Tracking on Fast Steering Mirror and Control Strategy
NASA Astrophysics Data System (ADS)
Di, Lin; Yi-ming, Wu; Fan, Zhu
2018-01-01
Fast steering mirror is a device used for controlling the beam direction precisely. Due to the short travel of the push-pull FSM, a compound fast steering mirror system driven by both limited-angle voice coil motor and push-pull FSM together is proposed. In the compound FSM system, limited-angle voice coil motor quickly swings at wide angle, while the push-pull FSM do high frequency movement in a small range, which provides the system with the high bandwidth and long travel. In the control strategy, the method of combining feed-forward control in Kalman filtering with auto-disturbance rejection control is used to improve trajectory tracking accuracy. The simulation result shows that tracking accuracy measured by the compound method can be improved by more than 5 times than that of the conventional PID.
An ultrafast angle-resolved photoemission apparatus for measuring complex materials
NASA Astrophysics Data System (ADS)
Smallwood, Christopher L.; Jozwiak, Christopher; Zhang, Wentao; Lanzara, Alessandra
2012-12-01
We present technical specifications for a high resolution time- and angle-resolved photoemission spectroscopy setup based on a hemispherical electron analyzer and cavity-dumped solid state Ti:sapphire laser used to generate pump and probe beams, respectively, at 1.48 and 5.93 eV. The pulse repetition rate can be tuned from 209 Hz to 54.3 MHz. Under typical operating settings the system has an overall energy resolution of 23 meV, an overall momentum resolution of 0.003 Å-1, and an overall time resolution of 310 fs. We illustrate the system capabilities with representative data on the cuprate superconductor Bi2Sr2CaCu2O8+δ. The descriptions and analyses presented here will inform new developments in ultrafast electron spectroscopy.
Integrated experimental setup for angle resolved photoemission spectroscopy of transuranic materials
DOE Office of Scientific and Technical Information (OSTI.GOV)
Graham, Kevin S.; Joyce, John J.; Durakiewicz, Tomasz
2013-09-15
We have developed the Angle Resolved Photoemission Spectroscopy (ARPES) system for transuranic materials. The ARPES transuranic system is an endstation upgrade to the Laser Plasma Light Source (LPLS) at Los Alamos National Laboratory. The LPLS is a tunable light source for photoemission with a photon energy range covering the vacuum ultraviolet (VUV) and soft x-ray regions (27–140 eV). The LPLS was designed and developed for transuranic materials. Transuranic photoemission is currently not permitted at the public synchrotrons worldwide in the VUV energy range due to sample encapsulation requirements. With the addition of the ARPES capability to the LPLS system theremore » is an excellent opportunity to explore new details centered on the electronic structure of actinide and transuranic materials.« less
Jin, Wencan; Yeh, Po -Chun; Zaki, Nader; ...
2015-03-17
We report the directly measured electronic structure of exfoliated monolayer molybdenum disulfide (MoS₂) using micrometer-scale angle-resolved photoemission spectroscopy. Measurements of both suspended and supported monolayer MoS₂ elucidate the effects of interaction with a substrate. Thus, a suggested relaxation of the in-plane lattice constant is found for both suspended and supported monolayer MoS₂ crystals. For suspended MoS₂, a careful investigation of the measured uppermost valence band gives an effective mass at Γ¯ and Κ¯ of 2.00m₀ and 0.43m₀, respectively. We also measure an increase in the band linewidth from the midpoint of Γ¯Κ¯ to the vicinity of Κ¯ and briefly discussmore » its possible origin.« less
Creel survey sampling designs for estimating effort in short-duration Chinook salmon fisheries
McCormick, Joshua L.; Quist, Michael C.; Schill, Daniel J.
2013-01-01
Chinook Salmon Oncorhynchus tshawytscha sport fisheries in the Columbia River basin are commonly monitored using roving creel survey designs and require precise, unbiased catch estimates. The objective of this study was to examine the relative bias and precision of total catch estimates using various sampling designs to estimate angling effort under the assumption that mean catch rate was known. We obtained information on angling populations based on direct visual observations of portions of Chinook Salmon fisheries in three Idaho river systems over a 23-d period. Based on the angling population, Monte Carlo simulations were used to evaluate the properties of effort and catch estimates for each sampling design. All sampling designs evaluated were relatively unbiased. Systematic random sampling (SYS) resulted in the most precise estimates. The SYS and simple random sampling designs had mean square error (MSE) estimates that were generally half of those observed with cluster sampling designs. The SYS design was more efficient (i.e., higher accuracy per unit cost) than a two-cluster design. Increasing the number of clusters available for sampling within a day decreased the MSE of estimates of daily angling effort, but the MSE of total catch estimates was variable depending on the fishery. The results of our simulations provide guidelines on the relative influence of sample sizes and sampling designs on parameters of interest in short-duration Chinook Salmon fisheries.
NASA Astrophysics Data System (ADS)
Huang, Kuo-Ting; Chen, Hsi-Chao; Lin, Ssu-Fan; Lin, Ke-Ming; Syue, Hong-Ye
2012-09-01
While tin-doped indium oxide (ITO) has been extensively applied in flexible electronics, the problem of the residual stress has many obstacles to overcome. This study investigated the residual stress of flexible electronics by the double beam shadow moiré interferometer, and focused on the precision improvement with phase shifting interferometry (PSI). According to the out-of-plane displacement equation, the theoretical error depends on the grating pitch and the angle between incident light and CCD. The angle error could be reduced to 0.03% by the angle shift of 10° as a result of the double beam interferometer was a symmetrical system. But the experimental error of the double beam moiré interferometer still reached to 2.2% by the noise of the vibration and interferograms. In order to improve the measurement precision, PSI was introduced to the double shadow moiré interferometer. Wavefront phase was reconstructed by the five interferograms with the Hariharan algorithm. The measurement results of standard cylinder indicating the error could be reduced from 2.2% to less than 1% with PSI. The deformation of flexible electronic could be reconstructed fast and calculated the residual stress with the Stoney correction formula. This shadow moiré interferometer with PSI could improve the precision of residual stress for flexible electronics.
Consistency of Lower-Body Dimensions Using Surface Landmarks and Simple Measurement Tools.
Caia, Johnpaul; Weiss, Lawrence W; Chiu, Loren Z F; Schilling, Brian K; Paquette, Max R
2016-09-01
Caia, J, Weiss, LW, Chiu, LZF, Schilling, BK, and Paquette, MR. Consistency of lower-body dimensions using surface landmarks and simple measurement tools. J Strength Cond Res 30(9): 2600-2608, 2016-Body dimensions may influence various types of physical performance. This study was designed to establish the reliability and precision of bilateral lower-body dimensions using surface anatomic landmarks and either sliding calipers or goniometry. Fifty university students (25 men and 25 women) were measured on 2 separate occasions separated by 48 or 72 hours. A small digital caliper was used to acquire longitudinal dimensions of the feet, whereas a larger broad-blade caliper was used to measure lower-limb, hip, and pelvic dimensions. Quadriceps angle (Q-angle) was determined through surface goniometry. Data for all foot and lower-limb dimensions were both reliable and precise (intraclass correlation coefficient (ICC) ≥0.72, SEM 0.1-0.5 cm). Measures of Q-angle were also reliable and precise (ICC ≥0.85, SEM 0.2-0.4°). Findings from this investigation demonstrate that lower-body dimensions may be reliably and precisely measured through simple practical tests, when surface anatomic landmarks and standardized procedures are used. Although intertester reliability remains to be established, meticulous adherence to specific measurement protocols is likely to yield viable output for lower-body dimensions when more sophisticated methods are unavailable or inappropriate.
Johnson, Jared M; Im, Soohyun; Windl, Wolfgang; Hwang, Jinwoo
2017-01-01
We propose a new scanning transmission electron microscopy (STEM) technique that can realize the three-dimensional (3D) characterization of vacancies, lighter and heavier dopants with high precision. Using multislice STEM imaging and diffraction simulations of β-Ga 2 O 3 and SrTiO 3 , we show that selecting a small range of low scattering angles can make the contrast of the defect-containing atomic columns substantially more depth-dependent. The origin of the depth-dependence is the de-channeling of electrons due to the existence of a point defect in the atomic column, which creates extra "ripples" at low scattering angles. The highest contrast of the point defect can be achieved when the de-channeling signal is captured using the 20-40mrad detection angle range. The effect of sample thickness, crystal orientation, local strain, probe convergence angle, and experimental uncertainty to the depth-dependent contrast of the point defect will also be discussed. The proposed technique therefore opens new possibilities for highly precise 3D structural characterization of individual point defects in functional materials. Copyright © 2016 Elsevier B.V. All rights reserved.
Speckle Interferometry at SOAR in 2016 and 2017
NASA Astrophysics Data System (ADS)
Tokovinin, Andrei; Mason, Brian D.; Hartkopf, William I.; Mendez, Rene A.; Horch, Elliott P.
2018-06-01
The results of speckle interferometric observations at the 4.1 m Southern Astrophysical Research Telescope in 2016 and 2017 are given, totaling 2483 measurements of 1570 resolved pairs and 609 non-resolutions. We describe briefly recent changes in the instrument and observing method and quantify the accuracy of the pixel scale and position angle calibration. Comments are given on 44 pairs resolved here for the first time. The orbital motion of the newly resolved subsystem BU 83 Aa,Ab roughly agrees with its 36-year astrometric orbit proposed by J. Dommanget. Most Tycho binaries examined here turned out to be spurious.
Rate-gyro-integral constraint for ambiguity resolution in GNSS attitude determination applications.
Zhu, Jiancheng; Li, Tao; Wang, Jinling; Hu, Xiaoping; Wu, Meiping
2013-06-21
In the field of Global Navigation Satellite System (GNSS) attitude determination, the constraints usually play a critical role in resolving the unknown ambiguities quickly and correctly. Many constraints such as the baseline length, the geometry of multi-baselines and the horizontal attitude angles have been used extensively to improve the performance of ambiguity resolution. In the GNSS/Inertial Navigation System (INS) integrated attitude determination systems using low grade Inertial Measurement Unit (IMU), the initial heading parameters of the vehicle are usually worked out by the GNSS subsystem instead of by the IMU sensors independently. However, when a rotation occurs, the angle at which vehicle has turned within a short time span can be measured accurately by the IMU. This measurement will be treated as a constraint, namely the rate-gyro-integral constraint, which can aid the GNSS ambiguity resolution. We will use this constraint to filter the candidates in the ambiguity search stage. The ambiguity search space shrinks significantly with this constraint imposed during the rotation, thus it is helpful to speeding up the initialization of attitude parameters under dynamic circumstances. This paper will only study the applications of this new constraint to land vehicles. The impacts of measurement errors on the effect of this new constraint will be assessed for different grades of IMU and current average precision level of GNSS receivers. Simulations and experiments in urban areas have demonstrated the validity and efficacy of the new constraint in aiding GNSS attitude determinations.
Signature of chaos in the 4 f -core-excited states for highly-charged tungsten ions
NASA Astrophysics Data System (ADS)
Safronova, Ulyana; Safronova, Alla
2014-05-01
We evaluate radiative and autoionizing transition rates in highly charged W ions in search for the signature of chaos. In particularly, previously published results for Ag-like W27+, Tm-like W5+, and Yb-like W4+ ions as well as newly obtained for I-like W21+, Xe-like W20+, Cs-like W19+, and La-like W17+ ions (with ground configuration [Kr] 4d10 4fk with k = 7, 8, 9, and 11, respectively) are considered that were calculated using the multiconfiguration relativistic Hebrew University Lawrence Livermore Atomic Code (HULLAC code) and the Hartree-Fock-Relativistic method (COWAN code). The main emphasis was on verification of Gaussian statistics of rates as a function of transition energy. There was no evidence of such statistics for above mentioned previously published results as well as for the transitions between the excited and autoionizing states for newly calculated results. However, we did find the Gaussian profile for the transitions between excited states such as the [Kr] 4d10 4fk - [Kr] 4d10 4f k - 1 5 d transitions , for newly calculated W ions. This work is supported in part by DOE under NNSA Cooperative Agreement DE-NA0001984.
van der Loop, Tibert H; Panman, Matthijs R; Lotze, Stephan; Zhang, Jing; Vad, Thomas; Bakker, Huib J; Sager, Wiebke F C; Woutersen, Sander
2012-07-28
We study the structure and reorientation dynamics of nanometer-sized water droplets inside nonionic reverse micelles (water/Igepal-CO-520/cyclohexane) with time-resolved mid-infrared pump-probe spectroscopy and small angle x-ray scattering. In the time-resolved experiments, we probe the vibrational and orientational dynamics of the O-D bonds of dilute HDO:H(2)O mixtures in Igepal reverse micelles as a function of temperature and micelle size. We find that even small micelles contain a large fraction of water that reorients at the same rate as water in the bulk, which indicates that the polyethylene oxide chains of the surfactant do not penetrate into the water volume. We also observe that the confinement affects the reorientation dynamics of only the first hydration layer. From the temperature dependent surface-water dynamics, we estimate an activation enthalpy for reorientation of 45 ± 9 kJ mol(-1) (11 ± 2 kcal mol(-1)), which is close to the activation energy of the reorientation of water molecules in ice.
Dakovski, Georgi L.; Durakiewicz, Tomasz; Zhu, Jian-Xin; ...
2015-10-12
A hallmark in the cuprate family of high-temperature superconductors is the nodal-antinodal dichotomy. In this regard, angle-resolved photoemission spectroscopy (ARPES) has proven especially powerful, providing band structure information directly in energy-momentum space. Time-resolved ARPES (trARPES) holds great promise of adding ultrafast temporal information, in an attempt to identify different interaction channels in the time domain. Previous studies of the cuprates using trARPES were handicapped by the low probing energy which significantly limits the accessible momentum space. Using 20.15eV, 12 fs pulses we show for the first time the evolution of quasiparticles in the antinodal region of Bi 2Sr 2CaCu 2Omore » 8+δ and demonstrate that nonmonotonic relaxation dynamics dominates above a certain fluence threshold. The dynamics is heavily influenced by transient modification of the electron-phonon interaction and phase space restrictions, in severe contrast to the monotonic relaxation in the nodal and off-nodal regions.« less
Horiba, K; Nakamura, Y; Nagamura, N; Toyoda, S; Kumigashira, H; Oshima, M; Amemiya, K; Senba, Y; Ohashi, H
2011-11-01
In order to achieve nondestructive observation of the three-dimensional spatially resolved electronic structure of solids, we have developed a scanning photoelectron microscope system with the capability of depth profiling in electron spectroscopy for chemical analysis (ESCA). We call this system 3D nano-ESCA. For focusing the x-ray, a Fresnel zone plate with a diameter of 200 μm and an outermost zone width of 35 nm is used. In order to obtain the angular dependence of the photoelectron spectra for the depth-profile analysis without rotating the sample, we adopted a modified VG Scienta R3000 analyzer with an acceptance angle of 60° as a high-resolution angle-resolved electron spectrometer. The system has been installed at the University-of-Tokyo Materials Science Outstation beamline, BL07LSU, at SPring-8. From the results of the line-scan profiles of the poly-Si/high-k gate patterns, we achieved a total spatial resolution better than 70 nm. The capability of our system for pinpoint depth-profile analysis and high-resolution chemical state analysis is demonstrated. © 2011 American Institute of Physics
Fourier-domain angle-resolved low coherence interferometry for clinical detection of dysplasia
NASA Astrophysics Data System (ADS)
Terry, Neil G.; Zhu, Yizheng; Wax, Adam
2010-02-01
Improved methods for detecting dysplasia, or pre-cancerous growth are a current clinical need, particularly in the esophagus. The currently accepted method of random biopsy and histological analysis provides only a limited examination of tissue in question while being coupled with a long time delay for diagnosis. Light scattering spectroscopy, in contrast, allows for inspection of the cellular structure and organization of tissue in vivo. Fourier-domain angle-resolved low-coherence interferometry (a/LCI) is a novel light scattering spectroscopy technique that provides quantitative depth-resolved morphological measurements of the size and optical density of the examined cell nuclei, which are characteristic biomarkers of dysplasia. Previously, clinical viability of the a/LCI system was demonstrated through analysis of ex vivo human esophageal tissue in Barrett's esophagus patients using a portable a/LCI, as was the development of a clinical a/LCI system. Data indicating the feasibility of the technique in other organ sites (colon, oral cavity) will be presented. We present an adaptation of the a/LCI system that will be used to investigate the presence of dysplasia in vivo in Barrett's esophagus patients.
Moskalensky, Alexander E; Yurkin, Maxim A; Konokhova, Anastasiya I; Strokotov, Dmitry I; Nekrasov, Vyacheslav M; Chernyshev, Andrei V; Tsvetovskaya, Galina A; Chikova, Elena D; Maltsev, Valeri P
2013-01-01
We introduce a novel approach for determination of volume and shape of individual blood platelets modeled as an oblate spheroid from angle-resolved light scattering with flow-cytometric technique. The light-scattering profiles (LSPs) of individual platelets were measured with the scanning flow cytometer and the platelet characteristics were determined from the solution of the inverse light-scattering problem using the precomputed database of theoretical LSPs. We revealed a phenomenon of parameter compensation, which is partly explained in the framework of anomalous diffraction approximation. To overcome this problem, additional a priori information on the platelet refractive index was used. It allowed us to determine the size of each platelet with subdiffraction precision and independent of the particular value of the platelet aspect ratio. The shape (spheroidal aspect ratio) distributions of platelets showed substantial differences between native and activated by 10 μM adenosine diphosphate samples. We expect that the new approach may find use in hematological analyzers for accurate measurement of platelet volume distribution and for determination of the platelet activation efficiency.
Detection of ferromagnetic target based on mobile magnetic gradient tensor system
NASA Astrophysics Data System (ADS)
Gang, Y. I. N.; Yingtang, Zhang; Zhining, Li; Hongbo, Fan; Guoquan, Ren
2016-03-01
Attitude change of mobile magnetic gradient tensor system critically affects the precision of gradient measurements, thereby increasing ambiguity in target detection. This paper presents a rotational invariant-based method for locating and identifying ferromagnetic targets. Firstly, unit magnetic moment vector was derived based on the geometrical invariant, such that the intermediate eigenvector of the magnetic gradient tensor is perpendicular to the magnetic moment vector and the source-sensor displacement vector. Secondly, unit source-sensor displacement vector was derived based on the characteristic that the angle between magnetic moment vector and source-sensor displacement is a rotational invariant. By introducing a displacement vector between two measurement points, the magnetic moment vector and the source-sensor displacement vector were theoretically derived. To resolve the problem of measurement noises existing in the realistic detection applications, linear equations were formulated using invariants corresponding to several distinct measurement points and least square solution of magnetic moment vector and source-sensor displacement vector were obtained. Results of simulation and principal verification experiment showed the correctness of the analytical method, along with the practicability of the least square method.
Weak-coupling superconductivity in a strongly correlated iron pnictide
Charnukha, A.; Post, K. W.; Thirupathaiah, S.; Pröpper, D.; Wurmehl, S.; Roslova, M.; Morozov, I.; Büchner, B.; Yaresko, A. N.; Boris, A. V.; Borisenko, S. V.; Basov, D. N.
2016-01-01
Iron-based superconductors have been found to exhibit an intimate interplay of orbital, spin, and lattice degrees of freedom, dramatically affecting their low-energy electronic properties, including superconductivity. Albeit the precise pairing mechanism remains unidentified, several candidate interactions have been suggested to mediate the superconducting pairing, both in the orbital and in the spin channel. Here, we employ optical spectroscopy (OS), angle-resolved photoemission spectroscopy (ARPES), ab initio band-structure, and Eliashberg calculations to show that nearly optimally doped NaFe0.978Co0.022As exhibits some of the strongest orbitally selective electronic correlations in the family of iron pnictides. Unexpectedly, we find that the mass enhancement of itinerant charge carriers in the strongly correlated band is dramatically reduced near the Γ point and attribute this effect to orbital mixing induced by pronounced spin-orbit coupling. Embracing the true band structure allows us to describe all low-energy electronic properties obtained in our experiments with remarkable consistency and demonstrate that superconductivity in this material is rather weak and mediated by spin fluctuations. PMID:26729630
Roles of nonlocal conductivity on spin Hall angle measurement
NASA Astrophysics Data System (ADS)
Chen, Kai; Zhang, Shufeng
2017-10-01
Spin Hall angle characterizes the rate of spin-charge current conversion and it has become one of the most important material parameters for spintronics physics and device application. A long-standing controversy is that the spin Hall angles for a given material measured by spin pumping and by spin Hall torque experiments are inconsistent and they could differ by as much as an order of magnitude. By using the linear response spin transport theory, we explicitly formulate the relation between the spin Hall angle and measured variables in different experiments. We find that the nonlocal conductivity inherited in the layered structure plays a key role to resolve conflicting values of the spin Hall angle. We provide a generalized scheme for extracting spin transport coefficients from experimental data.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Fallon, C., E-mail: colm.fallon5@mail.dcu.ie; Hayden, P.; Walsh, N.
We present the results of a time and space resolved optical-spectroscopic study of colliding plasmas formed at the front surfaces of flat and inclined Cu slab targets as a function of both the distance and the wedge angle between them for angles ranging from 100° to 180° (laterally colliding plasmas). The key parameters studied are stagnation layer density, temperature, duration, and kinetics of atomic/ionic spatial distributions and all have been found to vary significantly with wedge angle. It is found that the density and temperature of the stagnation layer decrease with increasing wedge angle. It is also found that themore » larger the wedge angle, the tighter and more well defined the stagnation layer formed.« less
On the analysis of time-of-flight spin-echo modulated dark-field imaging data
NASA Astrophysics Data System (ADS)
Sales, Morten; Plomp, Jeroen; Bouwman, Wim G.; Tremsin, Anton S.; Habicht, Klaus; Strobl, Markus
2017-06-01
Spin-Echo Modulated Small Angle Neutron Scattering with spatial resolution, i.e. quantitative Spin-Echo Dark Field Imaging, is an emerging technique coupling neutron imaging with spatially resolved quantitative small angle scattering information. However, the currently achieved relatively large modulation periods of the order of millimeters are superimposed to the images of the samples. So far this required an independent reduction and analyses of the image and scattering information encoded in the measured data and is involving extensive curve fitting routines. Apart from requiring a priori decisions potentially limiting the information content that is extractable also a straightforward judgment of the data quality and information content is hindered. In contrast we propose a significantly simplified routine directly applied to the measured data, which does not only allow an immediate first assessment of data quality and delaying decisions on potentially information content limiting further reduction steps to a later and better informed state, but also, as results suggest, generally better analyses. In addition the method enables to drop the spatial resolution detector requirement for non-spatially resolved Spin-Echo Modulated Small Angle Neutron Scattering.
Theory of Mach reflection of detonation at glancing incidence
DOE Office of Scientific and Technical Information (OSTI.GOV)
Bdzil, John Bohdan; Short, Mark
In this paper, we present a theory for Mach reflection of a detonation undergoing glancing incidence reflection off of a rigid wall. Our focus is on condensed-phase explosives, which we describe with a constant adiabatic gamma equation of state and an irreversible and either state-independent or weakly state-dependent reaction rate. We consider two detonation models: (1) the instantaneous reaction heat-release Chapman–Jouguet (CJ) limit and (2) the spatially resolved reaction heat-release Zeldovich–von Neumann–Dmore » $$\\ddot{Ø}$$ring (ZND) limit, where here we only consider that a small fraction of the detonation energy release is spatially resolved (the SRHR limit). We observe a three-shock reflection in the CJ limit case, with a Mach shock that is curved. In addition, we develop an analytical expression for the triple-point track angle as a function of the angle of incidence. For the SRHR model, we observe a smooth lead shock, akin to von Neumann reflection, with no reflected shock in the reaction zone. Only at larger angles of incidence is a three-shock Mach reflection observed.« less
Theory of Mach reflection of detonation at glancing incidence
Bdzil, John Bohdan; Short, Mark
2016-12-06
In this paper, we present a theory for Mach reflection of a detonation undergoing glancing incidence reflection off of a rigid wall. Our focus is on condensed-phase explosives, which we describe with a constant adiabatic gamma equation of state and an irreversible and either state-independent or weakly state-dependent reaction rate. We consider two detonation models: (1) the instantaneous reaction heat-release Chapman–Jouguet (CJ) limit and (2) the spatially resolved reaction heat-release Zeldovich–von Neumann–Dmore » $$\\ddot{Ø}$$ring (ZND) limit, where here we only consider that a small fraction of the detonation energy release is spatially resolved (the SRHR limit). We observe a three-shock reflection in the CJ limit case, with a Mach shock that is curved. In addition, we develop an analytical expression for the triple-point track angle as a function of the angle of incidence. For the SRHR model, we observe a smooth lead shock, akin to von Neumann reflection, with no reflected shock in the reaction zone. Only at larger angles of incidence is a three-shock Mach reflection observed.« less
Measurement of Thicknesses of High-κ Gate-Dielectric Films on Silicon by Angle-Resolved XPS
NASA Astrophysics Data System (ADS)
Powell, Cedric; Smekal, Werner; Werner, Wolfgang
2006-03-01
We report on the use of a new NIST database for the Simulation of Electron Spectra for Surface Analysis (SESSA) in measuring thicknesses of candidate high-κ gate-dielectric materials (HfO2, HfSiO4, ZrO2, and ZrSiO4) on silicon by angle-resolved XPS. For conventional measurements of film thicknesses, effective attenuation lengths (EALs) have been computed for these materials from SESSA as a function of film thickness and photoelectron emission angle (i.e., to simulate the effects of tilting the sample). These EALs are believed to be more accurate than similar EALs obtained from the transport approximation because realistic cross sections are used for both elastic and inelastic scattering in the film and substrate materials. We also present ``calibration curves'' showing calculated ratios of selected photoelectron intensities from thin films of HfO2 on Si with an intermediate SiO2 layer. These ratios provide a simple and convenient means of determining the thicknesses of SiO2 and HfO2 films for particular measurement conditions.
NASA Astrophysics Data System (ADS)
Zhou, Shudao; Ma, Zhongliang; Wang, Min; Peng, Shuling
2018-05-01
This paper proposes a novel alignment system based on the measurement of optical path using a light beam scanning mode in a transmissometer. The system controls both the probe beam and the receiving field of view while scanning in two vertical directions. The system then calculates the azimuth angle of the transmitter and the receiver to determine the precise alignment of the optical path. Experiments show that this method can determine the alignment angles in less than 10 min with errors smaller than 66 μrad in the azimuth. This system also features high collimation precision, process automation and simple installation.
Powerful Electromechanical Linear Actuator
NASA Technical Reports Server (NTRS)
Cowan, John R.; Myers, William N.
1994-01-01
Powerful electromechanical linear actuator designed to replace hydraulic actuator. Cleaner, simpler, and needs less maintenance. Features rotary-to-linear-motion converter with antibacklash gearing and position feedback via shaft-angle resolvers, which measure rotary motion.
Neutze, Richard; Moffat, Keith
2012-01-01
X-ray free electron lasers (XFELs) are potentially revolutionary X-ray sources because of their very short pulse duration, extreme peak brilliance and high spatial coherence, features that distinguish them from today’s synchrotron sources. We review recent time-resolved Laue diffraction and time-resolved wide angle X-ray scattering (WAXS) studies at synchrotron sources, and initial static studies at XFELs. XFELs have the potential to transform the field of time-resolved structural biology, yet many challenges arise in devising and adapting hardware, experimental design and data analysis strategies to exploit their unusual properties. Despite these challenges, we are confident that XFEL sources are poised to shed new light on ultrafast protein reaction dynamics. PMID:23021004
NASA Technical Reports Server (NTRS)
Hoge, F. E.; Swift, R. N.
1983-01-01
Airborne laser-induced, depth-resolved water Raman backscatter is useful in the detection and mapping of water optical transmission variations. This test, together with other field experiments, has identified the need for additional field experiments to resolve the degree of the contribution to the depth-resolved, Raman-backscattered signal waveform that is due to (1) sea surface height or elevation probability density; (2) off-nadir laser beam angle relative to the mean sea surface; and (3) the Gelbstoff fluorescence background, and the analytical techniques required to remove it. When converted to along-track profiles, the waveforms obtained reveal cells of a decreased Raman backscatter superimposed on an overall trend of monotonically decreasing water column optical transmission.
Hockett, Paul; Staniforth, Michael; Reid, Katharine L
2010-10-28
In this article we present photoelectron spectra and angular distributions in which ion rotational states are resolved. This data enables the comparison of direct and threshold photoionization techniques. We also present angle-resolved photoelectron signals at different total energies, providing a method to scan the structure of the continuum in the near-threshold region. Finally, we have studied the influence of vibrational excitation on the photoionization dynamics.
Innovative Techniques to Predict Atmospheric Effects on Sensor Performance
2009-10-15
since acquiring the MRO data, extensive tabulation of all of the data from all visible satellites (generally, non- resolved ) was also accomplished...efficient code has been written to run multiple OSC simulations in less time . Data from many passes of the same satellite is useful for SOI, whether it is...the data analyzed. Questions about the data were resolved using OSC to determine solar phase angle (SPA), range, time of penumbra entrance/exit and
Measurement of the Effective Weak Mixing Angle in p p ¯ → Z / γ * → e + e - Events
Abazov, V. M.; Abbott, B.; Acharya, B. S.; ...
2015-07-22
We present a measurement of the fundamental parameter of the standard model, the weak mixing angle sin 2θ ℓ eff which determines the relative strength of weak and electromagnetic interactions, in pp¯→Z/γ*→e +e - events at a center of mass energy of 1.96 TeV, using data corresponding to 9.7 fb -1 of integrated luminosity collected by the D0 detector at the Fermilab Tevatron. The effective weak mixing angle is extracted from the forward-backward charge asymmetry as a function of the invariant mass around the Z boson pole. The measured value of sin 2θ ℓ eff=0.23147±0.00047 is the most precise measurementmore » from light quark interactions to date, with a precision close to the best LEP and SLD results.« less
Measurement of the Effective Weak Mixing Angle in p p ¯ → Z / γ * → e + e - Events
DOE Office of Scientific and Technical Information (OSTI.GOV)
Abazov, V. M.; Abbott, B.; Acharya, B. S.
2015-07-22
We present a measurement of the fundamental parameter of the standard model, the weak mixing angle sin 2θ ℓ eff which determines the relative strength of weak and electromagnetic interactions, in pp¯→Z/γ*→e +e - events at a center of mass energy of 1.96 TeV, using data corresponding to 9.7 fb -1 of integrated luminosity collected by the D0 detector at the Fermilab Tevatron. The effective weak mixing angle is extracted from the forward-backward charge asymmetry as a function of the invariant mass around the Z boson pole. The measured value of sin 2θ ℓ eff=0.23147±0.00047 is the most precise measurementmore » from light quark interactions to date, with a precision close to the best LEP and SLD results.« less
Brault, C; Gil, C; Boboc, A; Spuig, P
2011-04-01
On the Tore Supra tokamak, a far infrared polarimeter diagnostic has been routinely used for diagnosing the current density by measuring the Faraday rotation angle. A high precision of measurement is needed to correctly reconstruct the current profile. To reach this precision, electronics used to compute the phase and the amplitude of the detected signals must have a good resilience to the noise in the measurement. In this article, the analogue card's response to the noise coming from the detectors and their impact on the Faraday angle measurements are analyzed, and we present numerical methods to calculate the phase and the amplitude. These validations have been done using real signals acquired by Tore Supra and JET experiments. These methods have been developed to be used in real-time in the future numerical cards that will replace the Tore Supra present analogue ones. © 2011 American Institute of Physics
Array Of Sensors Measures Broadband Radiation
NASA Technical Reports Server (NTRS)
Hoffman, James W.; Grush, Ronald G.
1994-01-01
Multiple broadband radiation sensors aimed at various portions of total field of view. All sensors mounted in supporting frame, serving as common heat sink and temperature reference. Each sensor includes heater winding and differential-temperature-sensing bridge circuit. Power in heater winding adjusted repeatedly in effort to balance bridge circuit. Intended to be used aboard satellite in orbit around Earth to measure total radiation emitted, at various viewing angles, by mosaic of "footprint" areas (each defined by its viewing angle) on surface of Earth. Modified versions of array useful for angle-resolved measurements of broadband radiation in laboratory and field settings on Earth.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Johannsen, Tim; Psaltis, Dimitrios
According to the no-hair theorem, astrophysical black holes are fully characterized by their masses and spins and are described by the Kerr metric. This theorem can be tested observationally by measuring (at least) three different multipole moments of the spacetimes of black holes. In this paper, we calculate the profiles of fluorescent iron lines emitted from the accretion flows around black hole candidates within a framework that allows us to perform the calculation as a function of its mass and spin as well as of a free parameter that measures potential deviations from the Kerr metric. We show that suchmore » deviations lead to line profiles that are significantly altered and may exhibit a modified flux ratio of the two peaks in their characteristic double-peaked shape. We also show that the disk inclination can be measured independently of the spin and the deviation parameter at low to intermediate inclination angles, as in the case of Kerr black holes. We estimate the precision that near-future X-ray missions such as Astro-H and ATHENA+ are required to achieve in order to resolve deviations from the Kerr metric in iron line profiles and show that constraints on such deviations will be strongest for rapidly spinning black holes. More generally, we show that measuring the line profile with a precision of {approx}5% at disk inclinations of 30 Degree-Sign or 60 Degree-Sign constrains the deviation parameter to order unity for values of the spin a {approx}> 0.5M.« less
Zheng, Yongbin; Chen, Huimin; Zhou, Zongtan
2018-05-23
The accurate angle measurement of objects outside the linear field of view (FOV) is a challenging task for a strapdown semi-active laser seeker and is not yet well resolved. Considering the fact that the strapdown semi-active laser seeker is equipped with GPS and an inertial navigation system (INS) on a missile, in this work, we present an angle measurement method based on the fusion of the seeker’s data and GPS and INS data for a strapdown semi-active laser seeker. When an object is in the nonlinear FOV or outside the FOV, by solving the problems of space consistency and time consistency, the pitch angle and yaw angle of the object can be calculated via the fusion of the last valid angles measured by the seeker and the corresponding GPS and INS data. The numerical simulation results demonstrate the correctness and effectiveness of the proposed method.
NASA Astrophysics Data System (ADS)
He, Qiuwei; Lv, Xingming; Wang, Xin; Qu, Xingtian; Zhao, Ji
2017-01-01
Blade is the key component in the energy power equipment of turbine, aircraft engines and so on. Researches on the process and equipment for blade finishing become one of important and difficult point. To control precisely tool system of developed hybrid grinding and polishing machine tool for blade finishing, the tool system with changeable wheel for belt polishing is analyzed in this paper. Firstly, the belt length and wrap angle of each wheel in different position of tension wheel swing angle in the process of changing wheel is analyzed. The reasonable belt length is calculated by using MATLAB, and relationships between wrap angle of each wheel and cylinder expansion amount of contact wheel are obtained. Then, the control system for changeable wheel tool structure is developed. Lastly, the surface roughness of blade finishing is verified by experiments. Theoretical analysis and experimental results show that reasonable belt length and wheel wrap angle can be obtained by proposed analysis method, the changeable wheel tool system can be controlled precisely, and the surface roughness of blade after grinding meets the design requirements.
NASA Astrophysics Data System (ADS)
Lindberg, P. A. P.; Shen, Z.-X.; Dessau, D. S.; Wells, B. O.; Mitzi, D. B.; Lindau, I.; Spicer, W. E.; Kapitulnik, A.
1989-09-01
Angle-resolved photoemission studies of single-crystalline La-doped Bi-Sr-Ca-Cu- 90-K superconductors (Bi2.0Sr1.8Ca0.8La0.3Cu2.1O8+δ) were performed utilizing synchrotron radiation covering the photon energy range 10-40 eV. The data conclusively reveal a dispersionless character of the valence-band states as a function of the wave-vector component parallel to the c axis, in agreement with the predictions of band calculations. Band effects are evident from both intensity modulations of the spectral features in the valence band and from energy dispersions as a function of the wave vector component lying in the basal a-b plane.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Gubbiotti, G.; Tacchi, S.; Montoncello, F.
2015-06-29
The Brillouin light scattering technique has been exploited to study the angle-resolved spin wave band diagrams of squared Permalloy antidot lattice. Frequency dispersion of spin waves has been measured for a set of fixed wave vector magnitudes, while varying the wave vector in-plane orientation with respect to the applied magnetic field. The magnonic band gap between the two most dispersive modes exhibits a minimum value at an angular position, which exclusively depends on the product between the selected wave vector magnitude and the lattice constant of the array. The experimental data are in very good agreement with predictions obtained bymore » dynamical matrix method calculations. The presented results are relevant for magnonic devices where the antidot lattice, acting as a diffraction grating, is exploited to achieve multidirectional spin wave emission.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Kimura, Shin-ichi; Ito, Takahiro; Nakamura, Eiken
A high-energy-resolution angle-resolved photoemission beamline in the vacuum-ultraviolet (VUV) region has been designed for a 750 MeV synchrotron light source UVSOR-II. The beamline equips an APPLE-II-type undulator with the horizontally/vertically linear and right/left circular polarizations, a modified Wadsworth-type monochromator and a high-resolution photoelectron analyzer. The monochromator covers the photon energy range of 6 - 40 eV. The energy resolution (hv/{delta}hv) and the photon flux on samples are expected to be 2 x 104 and 1012 photons/sec at 10 eV, 4 x 104 and 5 x 1011 photons/sec at 20 eV, and 6 x 104 and 1011 photons/sec at 40 eV,more » respectively. The beamline provides the high-resolution angle-resolved photoemission spectroscopy less than 1 meV in the whole VUV energy range.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Graf, J.; d'Astuto, M.; Jozwiak, C.
We report the first measurement of the Cu-O bond stretching phonon dispersion in optimally doped Bi{sub 2}Sr{sub 1.6}La{sub 0.4}Cu{sub 2}O{sub 6+{delta}} using inelastic x-ray scattering. We found a softening of this phonon at q = ({approx} 0.25, 0, 0) from 76 to 60 meV, similar to the one reported in other cuprates. A comparison with angle-resolved photoemission data on the same sample revealed an excellent agreement in terms of energy and momentum between the angle-resolved photoemission nodal kink and the soft part of the bond stretching phonon. Indeed, we find that the momentum space where a 63 {+-} 5 meVmore » kink is observed can be connected with a vector q = ({zeta}, 0, 0) with {zeta} {ge} 0.22, corresponding exactly to the soft part of the bond stretching phonon.« less
NASA Astrophysics Data System (ADS)
Schröder, Sven; Gliech, Stefan; Duparré, Angela
2005-10-01
An instrumentation for total and angle-resolved scattering (ARS) at 193 and 157 nm has been developed at the Fraunhofer Institute in Jena to meet the severe requirements for scattering analysis of deep- and vacuum-ultraviolet optical components. Extremely low backscattering levels of 10^-6 for the total scattering measurements and more than 9 orders of magnitude dynamic range for ARS have been accomplished. Examples of application extend from the control of at-wavelength scattering losses of superpolished substrates with rms roughness as small as 0.1 nm to the detection of volume material scattering and the study into the scattering of multilayer coatings. In addition, software programs were developed to model the roughness-induced light scattering of substrates and thin-film coatings.
NASA Astrophysics Data System (ADS)
Hamamoto, Satoru; Fujioka, Shuhei; Kanai, Yuina; Yamagami, Kohei; Nakatani, Yasuhiro; Nakagawa, Koya; Fujiwara, Hidenori; Kiss, Takayuki; Higashiya, Atsushi; Yamasaki, Atsushi; Kadono, Toshiharu; Imada, Shin; Tanaka, Arata; Tamasaku, Kenji; Yabashi, Makina; Ishikawa, Tetsuya; Matsumoto, Keisuke T.; Onimaru, Takahiro; Takabatake, Toshiro; Sekiyama, Akira
2017-12-01
We report experimentally observed linear dichroism in angle-resolved core-level photoemission spectra of PrIr2Zn20 and PrB6 with cubic symmetry. The different anisotropic 4f charge distributions between the compounds due to the crystalline-electric-field splitting are responsible for the difference in the linear dichroism, which has been verified by spectral simulations with the full multiplet theory for a single-site Pr3+ ion with cubic symmetry. The observed linear dichroism and polarization-dependent spectra in two different photoelectron directions for PrIr2Zn20 are reproduced by theoretical analysis for the Γ3 ground state, whereas those of the Pr 3d and 4d core levels indicate the Γ5 ground state for PrB6.
Zhang, Wentao; Liu, Guodong; Meng, Jianqiao; Zhao, Lin; Liu, Haiyun; Dong, Xiaoli; Lu, Wei; Wen, J S; Xu, Z J; Gu, G D; Sasagawa, T; Wang, Guiling; Zhu, Yong; Zhang, Hongbo; Zhou, Yong; Wang, Xiaoyang; Zhao, Zhongxian; Chen, Chuangtian; Xu, Zuyan; Zhou, X J
2008-07-04
Laser-based angle-resolved photoemission spectroscopy measurements have been carried out on the high energy electron dynamics in Bi2Sr2CaCu2O8 high temperature superconductor. Our superhigh resolution data, momentum-dependent measurements, and complete analysis provide important information to judge the nature of the high energy dispersion and kink. Our results rule out the possibility that the high energy dispersion from the momentum distribution curve (MDC) may represent the true bare band as believed in previous studies. We also rule out the possibility that the high energy kink represents electron coupling with some high energy modes as proposed before. Through detailed MDC and energy distribution curve analyses, we propose that the high energy MDC dispersion may not represent intrinsic band structure.
NASA Astrophysics Data System (ADS)
Jo, Youngju; Jung, Jaehwang; Lee, Jee Woong; Shin, Della; Park, Hyunjoo; Nam, Ki Tae; Park, Ji-Ho; Park, Yongkeun
2014-05-01
Two-dimensional angle-resolved light scattering maps of individual rod-shaped bacteria are measured at the single-cell level. Using quantitative phase imaging and Fourier transform light scattering techniques, the light scattering patterns of individual bacteria in four rod-shaped species (Bacillus subtilis, Lactobacillus casei, Synechococcus elongatus, and Escherichia coli) are measured with unprecedented sensitivity in a broad angular range from -70° to 70°. The measured light scattering patterns are analyzed along the two principal axes of rod-shaped bacteria in order to systematically investigate the species-specific characteristics of anisotropic light scattering. In addition, the cellular dry mass of individual bacteria is calculated and used to demonstrate that the cell-to-cell variations in light scattering within bacterial species is related to the cellular dry mass and growth.
First aircraft experiment results with the wide-angle airborne laser ranging system
NASA Astrophysics Data System (ADS)
Bock, Olivier; Thom, Christian; Kasser, Michel
1999-12-01
The first aircraft experiment with the Wide-Angle Airborne Laser Ranging System has been conducted in May 1998 over an air base in France equipped with a network of 64 cub-corner retroreflectors. The ranging system was operated from the Avion de Recherche Atmospherique et de Teledetection of CNES/IGN/INSU. Data have been collected during two 4-hour flights. The paper describes the data processing methods and presents the first experimental results. The precision is of 2 cm on the difference of vertical coordinates from two sets of 3 X 103 distance measurements, which is consistent with simulations and a posteriori covariance. The precision is mainly limited by the smallness of the number of efficient measurements remaining after a drastic data sorting for outliers. Higher precision is expected for future experiments after some instrumental improvements (achieving higher link budget) and measurement of aircraft attitude during the flight.
High-precision tracking of brownian boomerang colloidal particles confined in quasi two dimensions.
Chakrabarty, Ayan; Wang, Feng; Fan, Chun-Zhen; Sun, Kai; Wei, Qi-Huo
2013-11-26
In this article, we present a high-precision image-processing algorithm for tracking the translational and rotational Brownian motion of boomerang-shaped colloidal particles confined in quasi-two-dimensional geometry. By measuring mean square displacements of an immobilized particle, we demonstrate that the positional and angular precision of our imaging and image-processing system can achieve 13 nm and 0.004 rad, respectively. By analyzing computer-simulated images, we demonstrate that the positional and angular accuracies of our image-processing algorithm can achieve 32 nm and 0.006 rad. Because of zero correlations between the displacements in neighboring time intervals, trajectories of different videos of the same particle can be merged into a very long time trajectory, allowing for long-time averaging of different physical variables. We apply this image-processing algorithm to measure the diffusion coefficients of boomerang particles of three different apex angles and discuss the angle dependence of these diffusion coefficients.
Extending interferometric synthetic aperture radar measurements from one to two dimensions
NASA Astrophysics Data System (ADS)
Bechor, Noah
Interferometric synthetic aperture radar (InSAR), a very effective technique for measuring crustal deformation, provides measurements in only one dimension, along the radar line of sight. Imaging radar measurements from satellite-based systems are sensitive to both vertical and across-track displacements, but insensitive to along-track displacement. Multiple observations can resolve the first two components, but the along-track component remains elusive. The best existing method to obtain the along-track displacement involves pixel-level azimuth cross-correlation. The measurements are quite coarse (typically 15 cm precision), and they require large computation times. In contrast, across-track and vertical InSAR measurements can reach centimeter-level precision and are readily derived. We present a new method to extract along-track displacements from InSAR data. The new method, multiple aperture InSAR (MAI), is based on split-beam processing of InSAR data to create forward- and backward-looking interferograms. The phase difference between the two modified interferograms provides the along-track displacement component. Thus, from each conventional InSAR pair we extract two components of the displacement vector: one along the line of sight, the other in the along-track direction. Multiple MAI observations, either at two look angles or from the ascending and descending radar passes, then yield the three-dimensional displacement field. We analyze precision of our method by comparing our solution to GPS and offset-derived along-track displacements from interferograms of the M7.1 1999, Hector Mine earthquake. The RMS error between GPS displacements and our results ranges from 5 to 8.8cm. Our method is consistent with along-track displacements derived by pixel-offsets, themselves limited to 12-15cm precision. The theoretical MAI precision depends on SNR and coherence. For SNR=100 the expected precision is 3, 11cm for coherence of 0.8, 0.4, respectively. Finally, we evaluate how the new measurements improve the determination of the earthquake coseismic slip distribution by comparison of models derived from multiple data types. We find that MAI data help constrain the southern portion of the lip distribution, by adding information where GPS data are sparse and the deformation is below the azimuth pixel-offsets detection threshold.
Nundy, Surajit; Lotto, Beau; Coppola, David; Shimpi, Amita; Purves, Dale
2000-01-01
Although it has long been apparent that observers tend to overestimate the magnitude of acute angles and underestimate obtuse ones, there is no consensus about why such distortions are seen. Geometrical modeling combined with psychophysical testing of human subjects indicates that these misperceptions are the result of an empirical strategy that resolves the inherent ambiguity of angular stimuli by generating percepts of the past significance of the stimulus rather than the geometry of its retinal projection. PMID:10805814
Time-resolved optical spectrometer based on a monolithic array of high-precision TDCs and SPADs
NASA Astrophysics Data System (ADS)
Tamborini, Davide; Markovic, Bojan; Di Sieno, Laura; Contini, Davide; Bassi, Andrea; Tisa, Simone; Tosi, Alberto; Zappa, Franco
2013-12-01
We present a compact time-resolved spectrometer suitable for optical spectroscopy from 400 nm to 1 μm wavelengths. The detector consists of a monolithic array of 16 high-precision Time-to-Digital Converters (TDC) and Single-Photon Avalanche Diodes (SPAD). The instrument has 10 ps resolution and reaches 70 ps (FWHM) timing precision over a 160 ns full-scale range with a Differential Non-Linearity (DNL) better than 1.5 % LSB. The core of the spectrometer is the application-specific integrated chip composed of 16 pixels with 250 μm pitch, containing a 20 μm diameter SPAD and an independent TDC each, fabricated in a 0.35 μm CMOS technology. In front of this array a monochromator is used to focus different wavelengths into different pixels. The spectrometer has been used for fluorescence lifetime spectroscopy: 5 nm spectral resolution over an 80 nm bandwidth is achieved. Lifetime spectroscopy of Nile blue is demonstrated.
Metastable Autoionizing States of Molecules and Radicals in Highly Energetic Environment
2016-03-22
electronic states. The specific aims are to develop and calibrate complex-scaled equation-of-motion coupled cluster (cs-EOM- CC ) and CAP (complex...absorbing potential) augmented EOM- CC methods. We have implemented and benchmarked cs-EOM-CCSD and CAP- augmented EOM-CCSD methods for excitation energies...motion coupled cluster (cs-EOM- CC ) and CAP (complex absorbing potential) augmented EOM- CC methods. We have implemented and benchmarked cs-EOM-CCSD and
Resonant recombination and autoionization in electron-ion collisions
DOE Office of Scientific and Technical Information (OSTI.GOV)
Mueller, A.
1990-06-01
The occurence of resonances in elastic and inelastic electron-ion collisions is discussed. Resonant processes involve excitation of the ion with simultaneous capture of the initially free electron. The decay mechanism subsequent to the formation of the intermediate multiply excited state determines whether a resonance is found in recombination, excitation, elastic scattering, in single or even in multiple ionization. This review concentrates on resonances in the ionization channel. Correlated two-electron transitions are considered.
Absolute photoionization cross sections of atomic oxygen
NASA Technical Reports Server (NTRS)
Samson, J. A. R.; Pareek, P. N.
1982-01-01
The absolute values of photoionization cross sections of atomic oxygen were measured from the ionization threshold to 120 A. An auto-ionizing resonance belonging to the 2S2P4(4P)3P(3Do, 3So) transition was observed at 479.43 A and another line at 389.97 A. The experimental data is in excellent agreement with rigorous close-coupling calculations that include electron correlations in both the initial and final states.
Absolute photoionization cross sections of atomic oxygen
NASA Technical Reports Server (NTRS)
Samson, J. A. R.; Pareek, P. N.
1985-01-01
The absolute values of photoionization cross sections of atomic oxygen were measured from the ionization threshold to 120 A. An auto-ionizing resonance belonging to the 2S2P4(4P)3P(3Do, 3So) transition was observed at 479.43 A and another line at 389.97 A. The experimental data is in excellent agreement with rigorous close-coupling calculations that include electron correlations in both the initial and final states.
USDA-ARS?s Scientific Manuscript database
Cox (2010) reported that under business as usual, the environmental impacts of nutrient losses from agriculture will not be resolved and that precision conservation and precision regulation are two mechanisms to reduce the environmental impacts of nutrient losses. This is in agreement with the rece...
NASA Astrophysics Data System (ADS)
Staier, Florian; Eipel, Heinz; Matula, Petr; Evsikov, Alexei V.; Kozubek, Michal; Cremer, Christoph; Hausmann, Michael
2011-09-01
With the development of novel fluorescence techniques, high resolution light microscopy has become a challenging technique for investigations of the three-dimensional (3D) micro-cosmos in cells and sub-cellular components. So far, all fluorescence microscopes applied for 3D imaging in biosciences show a spatially anisotropic point spread function resulting in an anisotropic optical resolution or point localization precision. To overcome this shortcoming, micro axial tomography was suggested which allows object tilting on the microscopic stage and leads to an improvement in localization precision and spatial resolution. Here, we present a miniaturized device which can be implemented in a motor driven microscope stage. The footprint of this device corresponds to a standard microscope slide. A special glass fiber can manually be adjusted in the object space of the microscope lens. A stepwise fiber rotation can be controlled by a miniaturized stepping motor incorporated into the device. By means of a special mounting device, test particles were fixed onto glass fibers, optically localized with high precision, and automatically rotated to obtain views from different perspective angles under which distances of corresponding pairs of objects were determined. From these angle dependent distance values, the real 3D distance was calculated with a precision in the ten nanometer range (corresponding here to an optical resolution of 10-30 nm) using standard microscopic equipment. As a proof of concept, the spindle apparatus of a mature mouse oocyte was imaged during metaphase II meiotic arrest under different perspectives. Only very few images registered under different rotation angles are sufficient for full 3D reconstruction. The results indicate the principal advantage of the micro axial tomography approach for many microscopic setups therein and also those of improved resolutions as obtained by high precision localization determination.
Störmer, M; Gabrisch, H; Horstmann, C; Heidorn, U; Hertlein, F; Wiesmann, J; Siewert, F; Rack, A
2016-05-01
X-ray mirrors are needed for beam shaping and monochromatization at advanced research light sources, for instance, free-electron lasers and synchrotron sources. Such mirrors consist of a substrate and a coating. The shape accuracy of the substrate and the layer precision of the coating are the crucial parameters that determine the beam properties required for various applications. In principal, the selection of the layer materials determines the mirror reflectivity. A single layer mirror offers high reflectivity in the range of total external reflection, whereas the reflectivity is reduced considerably above the critical angle. A periodic multilayer can enhance the reflectivity at higher angles due to Bragg reflection. Here, the selection of a suitable combination of layer materials is essential to achieve a high flux at distinct photon energies, which is often required for applications such as microtomography, diffraction, or protein crystallography. This contribution presents the current development of a Ru/C multilayer mirror prepared by magnetron sputtering with a sputtering facility that was designed in-house at the Helmholtz-Zentrum Geesthacht. The deposition conditions were optimized in order to achieve ultra-high precision and high flux in future mirrors. Input for the improved deposition parameters came from investigations by transmission electron microscopy. The X-ray optical properties were investigated by means of X-ray reflectometry using Cu- and Mo-radiation. The change of the multilayer d-spacing over the mirror dimensions and the variation of the Bragg angles were determined. The results demonstrate the ability to precisely control the variation in thickness over the whole mirror length of 500 mm thus achieving picometer-precision in the meter-range.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Störmer, M., E-mail: michael.stoermer@hzg.de; Gabrisch, H.; Horstmann, C.
2016-05-15
X-ray mirrors are needed for beam shaping and monochromatization at advanced research light sources, for instance, free-electron lasers and synchrotron sources. Such mirrors consist of a substrate and a coating. The shape accuracy of the substrate and the layer precision of the coating are the crucial parameters that determine the beam properties required for various applications. In principal, the selection of the layer materials determines the mirror reflectivity. A single layer mirror offers high reflectivity in the range of total external reflection, whereas the reflectivity is reduced considerably above the critical angle. A periodic multilayer can enhance the reflectivity atmore » higher angles due to Bragg reflection. Here, the selection of a suitable combination of layer materials is essential to achieve a high flux at distinct photon energies, which is often required for applications such as microtomography, diffraction, or protein crystallography. This contribution presents the current development of a Ru/C multilayer mirror prepared by magnetron sputtering with a sputtering facility that was designed in-house at the Helmholtz-Zentrum Geesthacht. The deposition conditions were optimized in order to achieve ultra-high precision and high flux in future mirrors. Input for the improved deposition parameters came from investigations by transmission electron microscopy. The X-ray optical properties were investigated by means of X-ray reflectometry using Cu- and Mo-radiation. The change of the multilayer d-spacing over the mirror dimensions and the variation of the Bragg angles were determined. The results demonstrate the ability to precisely control the variation in thickness over the whole mirror length of 500 mm thus achieving picometer-precision in the meter-range.« less
NASA Astrophysics Data System (ADS)
Li, Xinji; Hui, Mei; Zhao, Zhu; Liu, Ming; Dong, Liquan; Kong, Lingqin; Zhao, Yuejin
2018-05-01
A differential computation method is presented to improve the precision of calibration for coaxial reverse Hartmann test (RHT). In the calibration, the accuracy of the distance measurement greatly influences the surface shape test, as demonstrated in the mathematical analyses. However, high-precision absolute distance measurement is difficult in the calibration. Thus, a differential computation method that only requires the relative distance was developed. In the proposed method, a liquid crystal display screen successively displayed two regular dot matrix patterns with different dot spacing. In a special case, images on the detector exhibited similar centroid distributions during the reflector translation. Thus, the critical value of the relative displacement distance and the centroid distributions of the dots on the detector were utilized to establish the relationship between the rays at certain angles and the detector coordinates. Experiments revealed the approximately linear behavior of the centroid variation with the relative displacement distance. With the differential computation method, we increased the precision of traditional calibration 10-5 rad root mean square. The precision of the RHT was increased by approximately 100 nm.
Design of automatic leveling and centering system of theodolite
NASA Astrophysics Data System (ADS)
Liu, Chun-tong; He, Zhen-Xin; Huang, Xian-xiang; Zhan, Ying
2012-09-01
To realize the theodolite automation and improve the azimuth Angle measurement instrument, the theodolite automatic leveling and centering system with the function of leveling error compensation is designed, which includes the system solution, key components selection, the mechanical structure of leveling and centering, and system software solution. The redesigned leveling feet are driven by the DC servo motor; and the electronic control center device is installed. Using high precision of tilt sensors as horizontal skew detection sensors ensures the effectiveness of the leveling error compensation. Aiming round mark center is located using digital image processing through surface array CCD; and leveling measurement precision can reach the pixel level, which makes the theodolite accurate centering possible. Finally, experiments are conducted using the automatic leveling and centering system of the theodolite. The results show the leveling and centering system can realize automatic operation with high centering accuracy of 0.04mm.The measurement precision of the orientation angle after leveling error compensation is improved, compared with that of in the traditional method. Automatic leveling and centering system of theodolite can satisfy the requirements of the measuring precision and its automation.
Refraction corrections for surveying
NASA Technical Reports Server (NTRS)
Lear, W. M.
1979-01-01
Optical measurements of range and elevation angle are distorted by the earth's atmosphere. High precision refraction correction equations are presented which are ideally suited for surveying because their inputs are optically measured range and optically measured elevation angle. The outputs are true straight line range and true geometric elevation angle. The 'short distances' used in surveying allow the calculations of true range and true elevation angle to be quickly made using a programmable pocket calculator. Topics covered include the spherical form of Snell's Law; ray path equations; and integrating the equations. Short-, medium-, and long-range refraction corrections are presented in tables.
NASA Astrophysics Data System (ADS)
Heilmann, Ralf K.; Bruccoleri, Alexander; Schattenburg, Mark; Kolodziejczak, jeffery; Gaskin, Jessica; O'Dell, Stephen L.
2017-01-01
A number of high priority subjects in astrophysics are addressed by a state-of-the-art soft x-ray grating spectrometer, e.g. the role of Active Galactic Nuclei in galaxy and star formation, characterization of the WHIM and the “missing baryon” problem, characterization of halos around the Milky Way and nearby galaxies, and stellar coronae and surrounding winds and disks. An Explorer-scale, large-area (A > 1,000 cm2), high resolving power (R > 3,000) soft x-ray grating spectrometer is highly feasible based on Critical-Angle Transmission (CAT) grating technology, even for telescopes with angular resolution of 5-10 arcsec. Significantly higher performance could be provided by a CAT grating spectrometer on an X-ray-Surveyor-type mission (A > 4,000 cm2, R > 5,000). CAT gratings combine advantages of blazed reflection gratings (high efficiency, use of higher orders) with those of transmission gratings (low mass, relaxed alignment tolerances and temperature requirements, transparent at higher energies) with minimal mission resource requirements. Blazing is achieved through grazing-incidence reflection off the smooth silicon grating bar sidewalls. Silicon is well matched to the soft x-ray band, and 30% absolute diffraction efficiency has been acheived with clear paths for further improvement. CAT gratings with sidewalls made of high-Z elements allow extension of blazing to higher energies and larger dispersion angles, enabling higher resolving power at shorter wavelengths. X-ray data from CAT gratings coated with a thin layer of platinum using atomic layer deposition demonstrate efficient blazing to higher energies and much larger blaze angles than possible with silicon alone. Measurements of the resolving power of a breadboard CAT grating spectrometer consisting of a Wolter-I slumped-glass focusing optic from GSFC and CAT gratings, taken at the MSFC Stray Light Facility, have demonstrated resolving power > 10,000. Thus currently fabricated CAT gratings are compatible with the most advanced grating spectrometer instrument designs for future soft x-ray spectroscopy missions. We will review the most recent CAT grating fabrication and x-ray test results.
Resolving runaway electron distributions in space, time, and energy
NASA Astrophysics Data System (ADS)
Paz-Soldan, C.; Cooper, C. M.; Aleynikov, P.; Eidietis, N. W.; Lvovskiy, A.; Pace, D. C.; Brennan, D. P.; Hollmann, E. M.; Liu, C.; Moyer, R. A.; Shiraki, D.
2018-05-01
Areas of agreement and disagreement with present-day models of runaway electron (RE) evolution are revealed by measuring MeV-level bremsstrahlung radiation from runaway electrons (REs) with a pinhole camera. Spatially resolved measurements localize the RE beam, reveal energy-dependent RE transport, and can be used to perform full two-dimensional (energy and pitch-angle) inversions of the RE phase-space distribution. Energy-resolved measurements find qualitative agreement with modeling on the role of collisional and synchrotron damping in modifying the RE distribution shape. Measurements are consistent with predictions of phase-space attractors that accumulate REs, with non-monotonic features observed in the distribution. Temporally resolved measurements find qualitative agreement with modeling on the impact of collisional and synchrotron damping in varying the RE growth and decay rate. Anomalous RE loss is observed and found to be largest at low energy. Possible roles for kinetic instability or spatial transport to resolve these anomalies are discussed.
Dynamic Measurement of Low Contact Angles by Optical Microscopy.
Campbell, James M; Christenson, Hugo K
2018-05-16
Precise measurement of contact angles is an important challenge in surface science, in the design and characterization of materials and in many crystallization experiments. Here we present a novel technique for measuring the contact angles of droplets between about 2° and 30°, with the lowest experimental uncertainty at the lower end of this range, typically ±0.1°. The lensing effect of a droplet interface produces the appearance of bright circles in low-aperture light, whose diameter is related to the contact angle. The technique requires no specialized equipment beyond an ordinary optical microscope, and may be used to study the dynamic evolution of the contact angle in situ during an experiment.
Shear Bond Strength of Bracket Bases to Adhesives Based on Bracket Base Design
2016-04-13
moving in the right direction. And to my wife, Allyson, I’m forever grateful for your patience and support, enabling me to pursue dreams as we begin... intrusion and extrusion in Angle and post Angle eras. As a result, the strength and precision of systems to apply forces through teeth have also
Multibeam collimator uses prism stack
NASA Technical Reports Server (NTRS)
Minott, P. O.
1981-01-01
Optical instrument creates many divergent light beams for surveying and machine element alignment applications. Angles and refractive indices of stack of prisms are selected to divert incoming laser beam by small increments, different for each prism. Angles of emerging beams thus differ by small, precisely-controlled amounts. Instrument is nearly immune to vibration, changes in gravitational force, temperature variations, and mechanical distortion.
NASA Technical Reports Server (NTRS)
Page, Norman A.; Tubbs, Eldred F.
1994-01-01
Retroreflectors made of concentric spherical optical elements developed for use in interferometric metrological systems. Used to provide reference point on structure to be aligned precisely in two or three dimensions by use of intersecting laser beams. Acceptance angle much larger than that of cat's-eye or corner-cube retroreflector: Simultaneously reflects laser beams separated by angles as large as 180 degrees.
VLBI geodesy - 2 parts-per-billion precision in length determinations for transcontinental baselines
NASA Technical Reports Server (NTRS)
Davis, J. L.; Herring, T. A.; Shapiro, I. I.
1988-01-01
VLBI was to make twenty-two independent measurements, between September 1984 and December 1986, of the length of the 3900-km baseline between the Mojave site in California and the Haystack/Westford site in Massachusetts. These experiments differ from the typical geodetic VLBI experiments in that a large fraction of observations is obtained at elevation angles between 4 and 10 deg. Data from these low elevation angles allow the vertical coordinate of site position, and hence the baseline length, to be estimated with greater precision. For the sixteen experiments processed thus far, the weighted root-mean-square scatter of the estimates of the baseline length is 8 mm.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Safronova, U. I.; Safronova, A. S.; Beiersdorfer, P.
Energy levels, radiative transition probabilities, and autoionization rates for [Ni]more » $$4{s}^{2}4{p}^{6}{nl}$$, [Ni]$$4{s}^{2}4{p}^{5}4l^{\\prime} {nl}$$ ($$l^{\\prime} =d,f,n$$ = 4–7), [Ni]$$4s4{p}^{6}4l^{\\prime} {nl}$$, ($$l^{\\prime} =d,f,n$$ = 4–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} {nl}$$ (n = 5–7), and [Ni]$$4s4{p}^{6}6l^{\\prime} {nl}$$ (n = 6–7) states in Rb-like tungsten (W37+) are calculated using the relativistic many-body perturbation theory method (RMBPT code) and the Hartree–Fock-relativistic method (COWAN code). Autoionizing levels above the [Ni]$$4{s}^{2}4{p}^{6}$$ threshold are considered. It is found that configuration mixing among [Ni]$$4{s}^{2}4{p}^{5}4l^{\\prime} {nl}$$ and [Ni]$$4s4{p}^{6}4l^{\\prime} {nl}$$ plays an important role for all atomic characteristics. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and dielectronic recombination (DR) rate coefficients are determined for the [Ni]$$4{s}^{2}4{p}^{6}{nl}$$ (n = 4–7) singly excited states, as well as the [Ni]$$4{s}^{2}4{p}^{5}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{5}4{fnl}$$, [Ni]$$4s4{p}^{6}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{6}4{fnl}$$, (n = 4–6), and [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} 5l$$ doubly excited nonautoionizing states in Rb-like W37+ ion. Contributions from the [Ni]$$4s24{p}^{6}4{fnl}$$ (n = 6–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\\prime} {nl}$$ (n = 5–6), and [Ni]$$4{s}^{2}4{p}^{5}6l^{\\prime} {nl}$$ (n = 6–7) doubly excited autoionizing states are evaluated numerically. The high-n state (with n up to 500) contributions are very important for high temperatures. These contributions are determined by using a scaling procedure. Synthetic dielectronic satellite spectra from Rb-like W are simulated in a broad spectral range from 8 to 70 Å. Here, these calculations provide highly accurate values for a number of W 37+ properties useful for a variety of applications including for fusion applications.« less
Study on verifying the angle measurement performance of the rotary-laser system
NASA Astrophysics Data System (ADS)
Zhao, Jin; Ren, Yongjie; Lin, Jiarui; Yin, Shibin; Zhu, Jigui
2018-04-01
An angle verification method to verify the angle measurement performance of the rotary-laser system was developed. Angle measurement performance has a great impact on measuring accuracy. Although there is some previous research on the verification of angle measuring uncertainty for the rotary-laser system, there are still some limitations. High-precision reference angles are used in the study of the method, and an integrated verification platform is set up to evaluate the performance of the system. This paper also probes the error that has biggest influence on the verification system. Some errors of the verification system are avoided via the experimental method, and some are compensated through the computational formula and curve fitting. Experimental results show that the angle measurement performance meets the requirement for coordinate measurement. The verification platform can evaluate the uncertainty of angle measurement for the rotary-laser system efficiently.
Angle-independent VO2 Thin Film on Glass Fiber Cloth as a Soft-Smart-Mirror (SSM)
Cai, Nianjin; Zhang, Wang; Wang, Wanlin; Zhu, Yuchen; Zada, Imran; Gu, Jiajun; Liu, Qinglei; Su, Huilan; Guo, Cuiping; Zhang, Zhijian; Zhang, Jianzhong; Wu, Liping; Zhang, Di
2016-01-01
Designing materials with a negative feedback function is beneficial for achieving temperature regulation inside a greenhouse. VO2 has been studied extensively because of its low insulator-to-metal transition temperature (IMT). In this study, reflection changes during a VO2 phase transition were investigated. Glass fiber cloth was used as a substrate, as it is stable and soft. A VO2 thin film on a glass fiber cloth whose surface contained 96% V4+ and 4% V5+ was prepared using an inorganic sol-gels method. The insulator-to-metal transition temperature was decreased by 38 °C, which was observed from the reflection curve detected using an angle-resolved spectrometer. This decrease in IMT occurred mainly because of the presence of V5+, which causes destabilization of the monoclinic phase of VO2. When the greenhouse temperature was increased from 30 °C to 40 °C, the reflected intensity of VO2 on glass fiber cloth decreased by 22% for the wavelength range of 400 nm to 800 nm. In addition, the angle-independent property of the VO2 thin film was observed using an angle-resolved spectrometer. Owing to its thermo-reflective properties, the thin film can serve as a soft-smart-mirror (SSM) inside a greenhouse to stabilize the temperature, playing a negative feedback role. PMID:27849051
Angle-independent VO2 Thin Film on Glass Fiber Cloth as a Soft-Smart-Mirror (SSM)
NASA Astrophysics Data System (ADS)
Cai, Nianjin; Zhang, Wang; Wang, Wanlin; Zhu, Yuchen; Zada, Imran; Gu, Jiajun; Liu, Qinglei; Su, Huilan; Guo, Cuiping; Zhang, Zhijian; Zhang, Jianzhong; Wu, Liping; Zhang, Di
2016-11-01
Designing materials with a negative feedback function is beneficial for achieving temperature regulation inside a greenhouse. VO2 has been studied extensively because of its low insulator-to-metal transition temperature (IMT). In this study, reflection changes during a VO2 phase transition were investigated. Glass fiber cloth was used as a substrate, as it is stable and soft. A VO2 thin film on a glass fiber cloth whose surface contained 96% V4+ and 4% V5+ was prepared using an inorganic sol-gels method. The insulator-to-metal transition temperature was decreased by 38 °C, which was observed from the reflection curve detected using an angle-resolved spectrometer. This decrease in IMT occurred mainly because of the presence of V5+, which causes destabilization of the monoclinic phase of VO2. When the greenhouse temperature was increased from 30 °C to 40 °C, the reflected intensity of VO2 on glass fiber cloth decreased by 22% for the wavelength range of 400 nm to 800 nm. In addition, the angle-independent property of the VO2 thin film was observed using an angle-resolved spectrometer. Owing to its thermo-reflective properties, the thin film can serve as a soft-smart-mirror (SSM) inside a greenhouse to stabilize the temperature, playing a negative feedback role.
Angle-independent VO2 Thin Film on Glass Fiber Cloth as a Soft-Smart-Mirror (SSM).
Cai, Nianjin; Zhang, Wang; Wang, Wanlin; Zhu, Yuchen; Zada, Imran; Gu, Jiajun; Liu, Qinglei; Su, Huilan; Guo, Cuiping; Zhang, Zhijian; Zhang, Jianzhong; Wu, Liping; Zhang, Di
2016-11-16
Designing materials with a negative feedback function is beneficial for achieving temperature regulation inside a greenhouse. VO 2 has been studied extensively because of its low insulator-to-metal transition temperature (IMT). In this study, reflection changes during a VO 2 phase transition were investigated. Glass fiber cloth was used as a substrate, as it is stable and soft. A VO 2 thin film on a glass fiber cloth whose surface contained 96% V 4+ and 4% V 5+ was prepared using an inorganic sol-gels method. The insulator-to-metal transition temperature was decreased by 38 °C, which was observed from the reflection curve detected using an angle-resolved spectrometer. This decrease in IMT occurred mainly because of the presence of V 5+ , which causes destabilization of the monoclinic phase of VO 2 . When the greenhouse temperature was increased from 30 °C to 40 °C, the reflected intensity of VO 2 on glass fiber cloth decreased by 22% for the wavelength range of 400 nm to 800 nm. In addition, the angle-independent property of the VO 2 thin film was observed using an angle-resolved spectrometer. Owing to its thermo-reflective properties, the thin film can serve as a soft-smart-mirror (SSM) inside a greenhouse to stabilize the temperature, playing a negative feedback role.
NASA Astrophysics Data System (ADS)
Zhang, Kexiong; Liao, Meiyong; Sumiya, Masatomo; Koide, Yasuo; Sang, Liwen
2016-11-01
The interfacial chemical state and the band alignment of the sputtering-deposited CaF2/p-GaN hetero-structure were investigated by angle-resolved X-ray photoelectron spectroscopy. The dependence of Ga 3p core-level positions on the collection angles proves that the downward band bending of p-GaN is reduced from 1.51 to 0.85 eV after the deposition of CaF2, which may be due to the reduction of Mg-Ga-O-related interface states by the oxygen-free deposition of CaF2. The band gap of sputtering-deposited CaF2 is estimated to be about 7.97 eV with a potential gradient of 0.48 eV obtained by the variation of the Ca 2p3/2 position on different collection angles. By taking into account the p-GaN surface band bending and potential gradient in the CaF2 layer, large valence and conduction band offsets of 2.66 ± 0.20 and 1.92 ± 0.20 eV between CaF2 and p-GaN are obtained. These results indicate that CaF2 is a promising gate dielectric layer on the p-GaN for the application of metal-insulator-semiconductor devices.
Yandayan, T; Geckeler, R D; Aksulu, M; Akgoz, S A; Ozgur, B
2016-05-01
The application of advanced error-separating shearing techniques to the precise calibration of autocollimators with Small Angle Generators (SAGs) was carried out for the first time. The experimental realization was achieved using the High Precision Small Angle Generator (HPSAG) of TUBITAK UME under classical dimensional metrology laboratory environmental conditions. The standard uncertainty value of 5 mas (24.2 nrad) reached by classical calibration method was improved to the level of 1.38 mas (6.7 nrad). Shearing techniques, which offer a unique opportunity to separate the errors of devices without recourse to any external standard, were first adapted by Physikalisch-Technische Bundesanstalt (PTB) to the calibration of autocollimators with angle encoders. It has been demonstrated experimentally in a clean room environment using the primary angle standard of PTB (WMT 220). The application of the technique to a different type of angle measurement system extends the range of the shearing technique further and reveals other advantages. For example, the angular scales of the SAGs are based on linear measurement systems (e.g., capacitive nanosensors for the HPSAG). Therefore, SAGs show different systematic errors when compared to angle encoders. In addition to the error-separation of HPSAG and the autocollimator, detailed investigations on error sources were carried out. Apart from determination of the systematic errors of the capacitive sensor used in the HPSAG, it was also demonstrated that the shearing method enables the unique opportunity to characterize other error sources such as errors due to temperature drift in long term measurements. This proves that the shearing technique is a very powerful method for investigating angle measuring systems, for their improvement, and for specifying precautions to be taken during the measurements.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Koh, S.K.; Song, S.K.; Choi, W.K.
A Kaufman-type 5 cm convex gridded ion-beam source is characterized in terms of angle-resolved ion-beam current density and beam uniformity at various discharge currents, electromagnet currents, and acceleration potentials. {copyright} {ital 1995} {ital American} {ital Institute} {ital of} {ital Physics}.
NASA Astrophysics Data System (ADS)
Watson, Matthew D.; Haghighirad, Amir A.; Rhodes, Luke C.; Hoesch, Moritz; Kim, Timur K.
2017-10-01
We report high resolution angle-resolved photo-emission spectroscopy (ARPES) measurements of detwinned FeSe single crystals. The application of a mechanical strain is used to promote the volume fraction of one of the orthorhombic domains in the sample, which we estimate to be 80 % detwinned. While the full structure of the electron pockets consisting of two crossed ellipses may be observed in the tetragonal phase at temperatures above 90 K, we find that remarkably, only one peanut-shaped electron pocket oriented along the longer a axis contributes to the ARPES measurement at low temperatures in the nematic phase, with the expected pocket along b being not observed. Thus the low temperature Fermi surface of FeSe as experimentally determined by ARPES consists of one elliptical hole pocket and one orthogonally-oriented peanut-shaped electron pocket. Our measurements clarify the long-standing controversies over the interpretation of ARPES measurements of FeSe.
Jobst, Johannes; van der Torren, Alexander J H; Krasovskii, Eugene E; Balgley, Jesse; Dean, Cory R; Tromp, Rudolf M; van der Molen, Sense Jan
2016-11-29
High electron mobility is one of graphene's key properties, exploited for applications and fundamental research alike. Highest mobility values are found in heterostructures of graphene and hexagonal boron nitride, which consequently are widely used. However, surprisingly little is known about the interaction between the electronic states of these layered systems. Rather pragmatically, it is assumed that these do not couple significantly. Here we study the unoccupied band structure of graphite, boron nitride and their heterostructures using angle-resolved reflected-electron spectroscopy. We demonstrate that graphene and boron nitride bands do not interact over a wide energy range, despite their very similar dispersions. The method we use can be generally applied to study interactions in van der Waals systems, that is, artificial stacks of layered materials. With this we can quantitatively understand the 'chemistry of layers' by which novel materials are created via electronic coupling between the layers they are composed of.
NASA Astrophysics Data System (ADS)
Rinott, Shahar; Ribak, Amit; Chashka, Khanan; Randeria, Mohit; Kanigel, Amit
The crossover from Bardeen-Cooper-Schrieffer (BCS) superconductivity to Bose-Einstein condensation (BEC) was never realized in quantum materials. It is difficult to realize because, unlike in ultra cold atoms, one cannot tune the pairing interaction. We realize the BCS-BEC crossover in a nearly compensated semimetal Fe1+ySexTe1-x by tuning the Fermi energy ɛF via chemical doping, which permits us to systematically change Δ /ɛF from 0 . 16 to 0 . 50 , where Δ is the superconducting (SC) gap. We use angle-resolved photoemission spectroscopy to measure the Fermi energy, the SC gap and characteristic changes in the SC state electronic dispersion as the system evolves from a BCS to a BEC regime. Our results raise important questions about the crossover in multi-band superconductors which go beyond those addressed in the context of cold atoms.
Gustavsen, Richard L.; Dattelbaum, Dana Mcgraw; Watkins, Erik Benjamin; ...
2017-03-10
Time resolved Small Angle X-ray Scattering (SAXS) experiments on detonating explosives have been conducted at Argonne National Laboratory's Advanced Photon Source Dynamic Compression Sector. The purpose of the experiments is to measure the SAXS patterns at tens of ns to a few μs behind the detonation front. Corresponding positions behind the detonation front are of order 0.1–10 mm. From the scattering patterns, properties of the explosive products relative to the time behind the detonation front can be inferred. Lastly, this report describes how the time and distance from the x-ray probe location to the detonation front is calculated, as wellmore » as the uncertainties and sources of uncertainty associated with the calculated times and distances.« less
Mahatha, S K; Patel, K D; Menon, Krishnakumar S R
2012-11-28
Angle-resolved photoemission spectroscopy (ARPES) and ab initio band structure calculations have been used to study the detailed valence band structure of molybdenite, MoS(2) and MoSe(2). The experimental band structure obtained from ARPES has been found to be in good agreement with the theoretical calculations performed using the linear augmented plane wave (LAPW) method. In going from MoS(2) to MoSe(2), the dispersion of the valence bands decreases along both k(parallel) and k(perpendicular), revealing the increased two-dimensional character which is attributed to the increasing interlayer distance or c/a ratio in these compounds. The width of the valence band and the band gap are also found to decrease, whereas the valence band maxima shift towards the higher binding energy from MoS(2) to MoSe(2).
DOE Office of Scientific and Technical Information (OSTI.GOV)
Ueoka, Y.; Ishikawa, Y.; Maejima, N.
2013-10-28
The electronic structures of amorphous indium gallium zinc oxide (a-IGZO) on a SiO{sub 2} layers before and after annealing were observed by constant final state X-ray photoelectron spectroscopy (CFS-XPS) and X-ray adsorption near-edge structure spectroscopy (XANES). From the results of angle-resolved CFS-XPS, the change in the electronic state was clearly observed in the a-IGZO bulk rather than in the a-IGZO/SiO{sub 2} interface. This suggests that the electronic structures of the a-IGZO bulk strongly affected the thin-film transistor characteristics. The results of XANES indicated an increase in the number of tail states upon atmospheric annealing (AT). We consider that the increasemore » in the number of tail states decreased the channel mobility of AT samples.« less
Zhang, W. -L.; Richard, P.; van Roekeghem, A.; ...
2016-10-31
We performed an angle-resolved photoemission spectroscopy study of BaMn 2As 2 and BaMn 2Sb 2, which are isostructural to the parent compound BaFe 2As 2 of the 122 family of ferropnictide superconductors. We show the existence of a strongly k z-dependent band gap with a minimum at the Brillouin zone center, in agreement with their semiconducting properties. Despite the half filling of the electronic 3d shell, we show that the band structure in these materials is almost not renormalized from the Kohn-Sham bands of density functional theory. Finally, our photon-energy-dependent study provides evidence for Mn-pnictide hybridization, which may play amore » role in tuning the electronic correlations in these compounds.« less
Theory of tunneling spectroscopy for chiral topological superconductors
NASA Astrophysics Data System (ADS)
Ii, Akihiro; Yamakage, Ai; Yada, Keiji; Sato, Masatoshi; Tanaka, Yukio
2012-11-01
We study the charge conductance of an interface between a normal metal and a superconducting quantum anomalous Hall system, based on the recursive Green's function. The angle-resolved conductance γ(ky,eV) with momentum ky parallel to the interface and bias voltage V shows a rich structure depending on the Chern number N of the system. We find that when the bias voltage is tuned to the energy dispersion of the edge mode, eV=Eedge(ky), the angle-resolved conductance γ(ky,Eedge(ky)) shows a pronounced even-odd effect; the conductance vanishes for N=0 or 2, while it takes the universal value 2e2/h for N=1. In particular, in the N=2 phase, we find that the conductance γ(ky,Eedge(ky)) becomes 0 due to the interference of two degenerate Majorana edge modes, although the corresponding surface spectral weight remains nonzero.
NASA Astrophysics Data System (ADS)
Fukahori, Shinichi; Ando, Toshiaki; Miura, Shun; Kanya, Reika; Yamanouchi, Kaoru; Rathje, Tim; Paulus, Gerhard G.
2017-05-01
The angle-resolved photoelectron spectra of Ar are recorded using intense circularly polarized near-infrared few-cycle laser pulses, and the effect of the depletion of Ar atoms by the ionization and the effect of the Coulombic potential are examined by the classical trajectory Monte Carlo simulations. On the basis of the comparison between the experimental and theoretical photoelectron spectra, a procedure for estimating the absolute carrier-envelope phase (CEP) of the few-cycle laser pulses interacting with atoms and molecules is proposed. It is confirmed that the absolute CEP can securely be estimated without any numerical calculations once the angular distribution of the yield of photoelectrons having the kinetic energy larger than 30 eV is measured with the peak laser intensity in the range between 1 ×1014 and 5 ×1014W /c m2 .
Pezzotti, Giuseppe; Zhu, Wenliang; Boffelli, Marco; Adachi, Tetsuya; Ichioka, Hiroaki; Yamamoto, Toshiro; Marunaka, Yoshinori; Kanamura, Narisato
2015-05-01
The Raman spectroscopic method has quantitatively been applied to the analysis of local crystallographic orientation in both single-crystal hydroxyapatite and human teeth. Raman selection rules for all the vibrational modes of the hexagonal structure were expanded into explicit functions of Euler angles in space and six Raman tensor elements (RTE). A theoretical treatment has also been put forward according to the orientation distribution function (ODF) formalism, which allows one to resolve the statistical orientation patterns of the nm-sized hydroxyapatite crystallite comprised in the Raman microprobe. Close-form solutions could be obtained for the Euler angles and their statistical distributions resolved with respect to the direction of the average texture axis. Polarized Raman spectra from single-crystalline hydroxyapatite and textured polycrystalline (teeth enamel) samples were compared, and a validation of the proposed Raman method could be obtained through confirming the agreement between RTE values obtained from different samples.
NASA Astrophysics Data System (ADS)
Jauernik, Stephan; Hein, Petra; Gurgel, Max; Falke, Julian; Bauer, Michael
2018-03-01
Laser-based angle-resolved photoelectron spectroscopy is performed on tin-phthalocyanine (SnPc) adsorbed on silver Ag(111). Upon adsorption of SnPc, strongly dispersing bands are observed which are identified as secondary Mahan cones formed by surface umklapp processes acting on photoelectrons from the silver substrate as they transit through the ordered adsorbate layer. We show that the photoemission data carry quantitative structural information on the adsorbate layer similar to what can be obtained from a conventional low-energy electron diffraction (LEED) study. More specifically, we compare photoemission data and LEED data probing an incommensurate-to-commensurate structural phase transition of the adsorbate layer. Based on our results we propose that Mahan-cone spectroscopy operated in a pump-probe configuration can be used in the future to probe structural dynamics at surfaces with a temporal resolution in the sub-100-fs regime.
NASA Astrophysics Data System (ADS)
Phan, G. N.; Nakayama, K.; Sugawara, K.; Sato, T.; Urata, T.; Tanabe, Y.; Tanigaki, K.; Nabeshima, F.; Imai, Y.; Maeda, A.; Takahashi, T.
2017-06-01
One of central issues in iron-based superconductors is the role of structural change to the superconducting transition temperature (Tc). It was found in FeSe that the lattice strain leads to a drastic increase in Tc, accompanied by suppression of nematic order. By angle-resolved photoemission spectroscopy on tensile- or compressive-strained and strain-free FeSe, we experimentally show that the in-plane strain causes a marked change in the energy overlap (Δ Eh -e ) between the hole and electron pockets in the normal state. The change in Δ Eh -e modifies the Fermi-surface volume, leading to a change in Tc. Furthermore, the strength of nematicity is also found to be characterized by Δ Eh -e . These results suggest that the key to understanding the phase diagram is the fermiology and interactions linked to the semimetallic band overlap.
Four-parameter model for polarization-resolved rough-surface BRDF.
Renhorn, Ingmar G E; Hallberg, Tomas; Bergström, David; Boreman, Glenn D
2011-01-17
A modeling procedure is demonstrated, which allows representation of polarization-resolved BRDF data using only four parameters: the real and imaginary parts of an effective refractive index with an added parameter taking grazing incidence absorption into account and an angular-scattering parameter determined from the BRDF measurement of a chosen angle of incidence, preferably close to normal incidence. These parameters allow accurate predictions of s- and p-polarized BRDF for a painted rough surface, over three decades of variation in BRDF magnitude. To characterize any particular surface of interest, the measurements required to determine these four parameters are the directional hemispherical reflectance (DHR) for s- and p-polarized input radiation and the BRDF at a selected angle of incidence. The DHR data describes the angular and polarization dependence, as well as providing the overall normalization constraint. The resulting model conserves energy and fulfills the reciprocity criteria.
Bidirectional reflectance distribution function effects in ladar-based reflection tomography.
Jin, Xuemin; Levine, Robert Y
2009-07-20
Light reflection from a surface is described by the bidirectional reflectance distribution function (BRDF). In this paper, BRDF effects in reflection tomography are studied using modeled range-resolved reflection from well-characterized geometrical surfaces. It is demonstrated that BRDF effects can cause a darkening at the interior boundary of the reconstructed surface analogous to the well-known beam hardening artifact in x-ray transmission computed tomography (CT). This artifact arises from reduced reflection at glancing incidence angles to the surface. It is shown that a purely Lambertian surface without shadowed components is perfectly reconstructed from range-resolved measurements. This result is relevant to newly fabricated carbon nanotube materials. Shadowing is shown to cause crossed streak artifacts similar to limited-angle effects in CT reconstruction. In tomographic reconstruction, these effects can overwhelm highly diffuse components in proximity to specularly reflecting elements. Diffuse components can be recovered by specialized processing, such as reducing glints via thresholded measurements.
NASA Astrophysics Data System (ADS)
Amorim, B.
2018-04-01
We develop a general theory to model the angle-resolved photoemission spectroscopy (ARPES) of commensurate and incommensurate van der Waals (vdW) structures, formed by lattice mismatched and/or misaligned stacked layers of two-dimensional materials. The present theory is based on a tight-binding description of the structure and the concept of generalized umklapp processes, going beyond previous descriptions of ARPES in incommensurate vdW structures, which are based on continuous, low-energy models, being limited to structures with small lattice mismatch/misalignment. As applications of the general formalism, we study the ARPES bands and constant energy maps for two structures: twisted bilayer graphene and twisted bilayer MoS2. The present theory should be useful in correctly interpreting experimental results of ARPES of vdW structures and other systems displaying competition between different periodicities, such as two-dimensional materials weakly coupled to a substrate and materials with density wave phases.
NASA Astrophysics Data System (ADS)
Liu, Guodong; Wang, Chenlu; Zhang, Yan; Hu, Bingfeng; Mou, Daixiang; Yu, Li; Zhao, Lin; Zhou, Xingjiang; Wang, Nanlin; Chen, Chuangtian; Xu, Zuyan
We performed high-resolution angle-resolved photoemission spectroscopy (ARPES) measurement on high quality crystal of HoTe3, an intriguing quasi-two-dimensional rare-earth-element tritelluride charge-density-wave (CDW) compound. The main features of the electronic structure in this compound are established by employing a quasi-CW laser (7eV) and a helium discharging lamp (21.22 eV) as excitation light sources. It reveals many bands back folded according to the CDW periodicity and two incommensurate CDW gaps created by perpendicular Fermi surface (FS) nesting vectors. A large gap is found to open in well nested regions of the Fermi surface sheets, whereas other Fermi surface sections with poor nesting remain ungapped. In particular, some peculiar features are identified by using our ultra-high resolution and bulk sensitive laser-ARPES.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Gustavsen, Richard L.; Dattelbaum, Dana Mcgraw; Watkins, Erik Benjamin
Time resolved Small Angle X-ray Scattering (SAXS) experiments on detonating explosives have been conducted at Argonne National Laboratory's Advanced Photon Source Dynamic Compression Sector. The purpose of the experiments is to measure the SAXS patterns at tens of ns to a few μs behind the detonation front. Corresponding positions behind the detonation front are of order 0.1–10 mm. From the scattering patterns, properties of the explosive products relative to the time behind the detonation front can be inferred. Lastly, this report describes how the time and distance from the x-ray probe location to the detonation front is calculated, as wellmore » as the uncertainties and sources of uncertainty associated with the calculated times and distances.« less
NASA Astrophysics Data System (ADS)
Silva, Norberto D., Jr.; Haydock, Christopher; Prendergast, Franklyn G.
1994-08-01
The time-resolved fluorescence decay of single tryptophan (Trp) proteins is typically described using either a distribution of lifetimes or a sum of two or more exponential terms. A possible interpretation for this fluorescence decay heterogeneity is the existence of different isomeric conformations of Trp about its (chi) +1) and (chi) +2) dihedral angles. Are multiple Trp conformations compatible with the remainder of the protein in its crystallographic configuration or do they require repacking of neighbor side chains? It is conceivable that isomers of the neighbor side chains interconvert slowly on the fluorescence timescale and contribute additional lifetime components to the fluorescence intensity. We have explored this possibility by performing minimum perturbation mapping simulations of Trp 28 and Trp 31 in thioredoxin (TRX) using CHARMm 22. Mappings of Trp 29 and Trp 31 give the TRX Trp residue energy landscape as a function of (chi) +1) and (chi) +2) dihedral angles. Time-resolved fluorescence intensity and anisotropy decay of mutant TRX (W28F and W31F) are measured and interpreted in light of the above simulations. Relevant observables, like order parameters and isomerization rates, can be derived from the minimum perturbation maps and compared with experiment.
High-angle-of-attack pneumatic lag and upwash corrections for a hemispherical flow direction sensor
NASA Technical Reports Server (NTRS)
Whitmore, Stephen A.; Heeg, Jennifer; Larson, Terry J.; Ehernberger, L. J.; Hagen, Floyd W.; Deleo, Richard V.
1987-01-01
As part of the NASA F-14 high angle of attack flight test program, a nose mounted hemispherical flow direction sensor was calibrated against a fuselage mounted movable vane flow angle sensor. Significant discrepancies were found to exist in the angle of attack measurements. A two fold approach taken to resolve these discrepancies during subsonic flight is described. First, the sensing integrity of the isolated hemispherical sensor is established by wind tunnel data extending to an angle of attack of 60 deg. Second, two probable causes for the discrepancies, pneumatic lag and upwash, are examined. Methods of identifying and compensating for lag and upwash are presented. The wind tunnel data verify that the isolated hemispherical sensor is sufficiently accurate for static conditions with angles of attack up to 60 deg and angles of sideslip up to 30 deg. Analysis of flight data for two high angle of attack maneuvers establishes that pneumatic lag and upwash are highly correlated with the discrepancies between the hemispherical and vane type sensor measurements.
Dual wavelength multiple-angle light scattering system for cryptosporidium detection
NASA Astrophysics Data System (ADS)
Buaprathoom, S.; Pedley, S.; Sweeney, S. J.
2012-06-01
A simple, dual wavelength, multiple-angle, light scattering system has been developed for detecting cryptosporidium suspended in water. Cryptosporidium is a coccidial protozoan parasite causing cryptosporidiosis; a diarrheal disease of varying severity. The parasite is transmitted by ingestion of contaminated water, particularly drinking-water, but also accidental ingestion of bathing-water, including swimming pools. It is therefore important to be able to detect these parasites quickly, so that remedial action can be taken to reduce the risk of infection. The proposed system combines multiple-angle scattering detection of a single and two wavelengths, to collect relative wavelength angle-resolved scattering phase functions from tested suspension, and multivariate data analysis techniques to obtain characterizing information of samples under investigation. The system was designed to be simple, portable and inexpensive. It employs two diode lasers (violet InGaN-based and red AlGaInP-based) as light sources and silicon photodiodes as detectors and optical components, all of which are readily available. The measured scattering patterns using the dual wavelength system showed that the relative wavelength angle-resolved scattering pattern of cryptosporidium oocysts was significantly different from other particles (e.g. polystyrene latex sphere, E.coli). The single wavelength set up was applied for cryptosporidium oocysts'size and relative refractive index measurement and differential measurement of the concentration of cryptosporidium oocysts suspended in water and mixed polystyrene latex sphere suspension. The measurement results showed good agreement with the control reference values. These results indicate that the proposed method could potentially be applied to online detection in a water quality control system.
Temporal Control and Hand Movement Efficiency in Skilled Music Performance
Goebl, Werner; Palmer, Caroline
2013-01-01
Skilled piano performance requires considerable movement control to accomplish the high levels of timing and force precision common among professional musicians, who acquire piano technique over decades of practice. Finger movement efficiency in particular is an important factor when pianists perform at very fast tempi. We document the finger movement kinematics of highly skilled pianists as they performed a five-finger melody at very fast tempi. A three-dimensional motion-capture system tracked the movements of finger joints, the hand, and the forearm of twelve pianists who performed on a digital piano at successively faster tempi (7–16 tones/s) until they decided to stop. Joint angle trajectories computed for all adjacent finger phalanges, the hand, and the forearm (wrist angle) indicated that the metacarpophalangeal joint contributed most to the vertical fingertip motion while the proximal and distal interphalangeal joints moved slightly opposite to the movement goal (finger extension). An efficiency measure of the combined finger joint angles corresponded to the temporal accuracy and precision of the pianists’ performances: Pianists with more efficient keystroke movements showed higher precision in timing and force measures. Keystroke efficiency and individual joint contributions remained stable across tempo conditions. Individual differences among pianists supported the view that keystroke efficiency is required for successful fast performance. PMID:23300946
Electronic structure of p-type transparent conducting oxide CuAlO2
NASA Astrophysics Data System (ADS)
Mo, Sung-Kwan; Yoon, Joonseok; Liu, Xiaosong; Yang, Wanli; Mun, Bongjin; Ju, Honglyoul
2014-03-01
CuAlO2 is a prototypical p-type transparent conducting oxide. Despite its importance for potential applications and number of studies on its band structure and gap characteristics, experimental study on the momentum-resolved electronic structure has been lacking. We present angle-resolved photoemission data on single crystalline CuAlO2 using synchrotron light source to reveal complete band structure. Complemented by the x-ray absorption and emission spectra, we also study band gap characteristics and compare them with theory.
Array-based satellite phase bias sensing: theory and GPS/BeiDou/QZSS results
NASA Astrophysics Data System (ADS)
Khodabandeh, A.; Teunissen, P. J. G.
2014-09-01
Single-receiver integer ambiguity resolution (IAR) is a measurement concept that makes use of network-derived non-integer satellite phase biases (SPBs), among other corrections, to recover and resolve the integer ambiguities of the carrier-phase data of a single GNSS receiver. If it is realized, the very precise integer ambiguity-resolved carrier-phase data would then contribute to the estimation of the receiver’s position, thus making (near) real-time precise point positioning feasible. Proper definition and determination of the SPBs take a leading part in developing the idea of single-receiver IAR. In this contribution, the concept of array-based between-satellite single-differenced (SD) SPB determination is introduced, which is aimed to reduce the code-dominated precision of the SD-SPB corrections. The underlying model is realized by giving the role of the local reference network to an array of antennas, mounted on rigid platforms, that are separated by short distances so that the same ionospheric delay is assumed to be experienced by all the antennas. To that end, a closed-form expression of the array-aided SD-SPB corrections is presented, thereby proposing a simple strategy to compute the SD-SPBs. After resolving double-differenced ambiguities of the array’s data, the variance of the SD-SPB corrections is shown to be reduced by a factor equal to the number of antennas. This improvement in precision is also affirmed by numerical results of the three GNSSs GPS, BeiDou and QZSS. Experimental results demonstrate that the integer-recovered ambiguities converge to integers faster, upon increasing the number of antennas aiding the SD-SPB corrections.
Metasurface Enabled Wide-Angle Fourier Lens.
Liu, Wenwei; Li, Zhancheng; Cheng, Hua; Tang, Chengchun; Li, Junjie; Zhang, Shuang; Chen, Shuqi; Tian, Jianguo
2018-06-01
Fourier optics, the principle of using Fourier transformation to understand the functionalities of optical elements, lies at the heart of modern optics, and it has been widely applied to optical information processing, imaging, holography, etc. While a simple thin lens is capable of resolving Fourier components of an arbitrary optical wavefront, its operation is limited to near normal light incidence, i.e., the paraxial approximation, which puts a severe constraint on the resolvable Fourier domain. As a result, high-order Fourier components are lost, resulting in extinction of high-resolution information of an image. Other high numerical aperture Fourier lenses usually suffer from the bulky size and costly designs. Here, a dielectric metasurface consisting of high-aspect-ratio silicon waveguide array is demonstrated experimentally, which is capable of performing 1D Fourier transform for a large incident angle range and a broad operating bandwidth. Thus, the device significantly expands the operational Fourier space, benefitting from the large numerical aperture and negligible angular dispersion at large incident angles. The Fourier metasurface will not only facilitate efficient manipulation of spatial spectrum of free-space optical wavefront, but also be readily integrated into micro-optical platforms due to its compact size. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
NASA Astrophysics Data System (ADS)
Kang, Ming; Zhu, Weiren; Rukhlenko, Ivan D.
2017-12-01
The exceptional point (EP), which is one of the most important branch-type singularities exclusive to non-Hermitian systems, has been observed recently in various synthetic materials, giving rise to counterintuitive phenomena due to the nontrivial topology of the EP. Here, we present a direct experimental observation of the topological structure of the EPs via the angle-resolved transmission measurement of a hybridized metamaterial. Both eigenvalues and eigenvectors show branch-point singularities in the investigated biparametric space of frequency and incident angle. Importantly, the angle-resolved transmission coefficients provide all the information about the eigenvalues as well as the corresponding eigenvectors in the biparametric space, revealing the nontrivial topological structure of the EP, such as mode switching and the topological phase for a parameter loop encircling the EP. It is shown that the appearance of the EP in the scattering matrix is related directly to the perfect unidirectional transmission and the chirality of the EP corresponds to the maximum or minimum value of the asymmetric factor. Our investigation uncovers the capabilities of metamaterials for exploring the physics of EPs and their potential for having extreme optical properties, which provide potential applications in the spectral band ranging from microwaves to visible frequencies.
Perkins, Bradford G; Nesbitt, David J
2007-08-09
Energy transfer dynamics at the gas-liquid interface have been probed with a supersonic molecular beam of CO2 and a clean perfluorinated-liquid surface in vacuum. High-resolution infrared spectroscopy measures both the rovibrational state populations and the translational distributions for the scattered CO2 flux. The present study investigates collision dynamics as a function of incident angle (thetainc = 0 degrees, 30 degrees, 45 degrees, and 60 degrees), where column-integrated quantum state populations are detected along the specular-scattering direction (i.e., thetascat approximately thetainc). Internal state rovibrational and Doppler translational distributions in the scattered CO2 yield clear evidence for nonstatistical behavior, providing quantum-state-resolved support for microscopic branching of the gas-liquid collision dynamics into multiple channels. Specifically, the data are remarkably well described by a two-temperature model, which can be associated with both a trapping desorption (TD) component emerging at the surface temperature (Trot approximately TS) and an impulsive scattering (IS) component appearing at hyperthermal energies (Trot > TS). The branching ratio between the TD and IS channels is found to depend strongly on thetainc, with the IS component growing dramatically with increasingly steeper angle of incidence.
Use of Yohkoh SXT in Measuring the Net Current and CME Productivity of Active Regions
NASA Technical Reports Server (NTRS)
Falconer, D. A.; Moore, R. L.; Gary, G. A.; Six, N. Frank (Technical Monitor)
2001-01-01
In our investigation of the correlation of global nonpotentiality of active regions to their CME productivity (Falconer, D.A. 2001, JGR, in press, and Falconer, Moore, & Gary, 2000, EOS 82, 20 S323), we use Yohkoh SXT images for two purposes. The first use is to help resolve the 180 degree ambiguity in the direction of the observed transverse magnetic field. Resolution of the 180 degree ambiguity is important, since the net current, one of our measures of global nonpotentiality, is derived from integrating the dot product of the transverse field around a contour (I(sub N)=(integral)BT(raised dot)dl). The ambiguity results from the observed transverse field being determined from the linear polarization, which gives the plane of the direction, but leaves a 180 degrees ambiguity. Automated methods to resolve the ambiguity ranging from the simple acute angle rule (Falconer, D.A. 2001) to the more sophisticated annealing method (Metcalf T.R. 1994). For many active regions, especially ones that are nearly potential these methods work well. But for very nonpotential active regions where the shear angle (the angle between the observed and potential transverse field) is near 90 degrees throughout large swaths along the main neutral line, both methods can resolve the ambiguity incorrectly for long segments of the neutral line. By determining from coronal images, such as those from Yohkoh/SXT, the sense of shear along the main neutral line in the active region, these cases can be identified and corrected by a modification of the acute angle rule described here. The second use of Yohkoh/SXT in this study is to check for the cusped coronal arcades of long-duration eruptive flares. This signature is an excellent proxy for CMEs, and was used by Canfield, Hudson, and McKenzie (1999 GRL V26, 6, 627-630). This work is funded by NSF through the Space Weather Program and by NASA through the Solar Physics Supporting Research and Technology Program.
Effect of the cosmological constant on the deflection angle by a rotating cosmic string
NASA Astrophysics Data System (ADS)
Jusufi, Kimet; Övgün, Ali
2018-03-01
We report the effect of the cosmological constant and the internal energy density of a cosmic string on the deflection angle of light in the spacetime of a rotating cosmic string with internal structure. We first revisit the deflection angle by a rotating cosmic string and then provide a generalization using the geodesic equations and the Gauss-Bonnet theorem. We show there is an agreement between the two methods when employing higher-order terms of the linear mass density of the cosmic string. By modifying the integration domain for the global conical topology, we resolve the inconsistency between these two methods previously reported in the literature. We show that the deflection angle is not affected by the rotation of the cosmic string; however, the cosmological constant Λ strongly affects the deflection angle, which generalizes the well-known result.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Dolphin, Andrew E., E-mail: adolphin@raytheon.com
The combination of spectroscopic stellar metallicities and resolved star color–magnitude diagrams (CMDs) has the potential to constrain the entire star formation history (SFH) of a galaxy better than fitting CMDs alone (as is most common in SFH studies using resolved stellar populations). In this paper, two approaches to incorporating external metallicity information into CMD-fitting techniques are presented. Overall, the joint fitting of metallicity and CMD information can increase the precision of measured age–metallicity relationships (AMRs) and star formation rates by 10% over CMD fitting alone. However, systematics in stellar isochrones and mismatches between spectroscopic and photometric determinations of metallicity canmore » reduce the accuracy of the recovered SFHs. I present a simple mitigation of these systematics that can reduce their amplitude to the level obtained from CMD fitting alone, while ensuring that the AMR is consistent with spectroscopic metallicities. As is the case in CMD-fitting analysis, improved stellar models and calibrations between spectroscopic and photometric metallicities are currently the primary impediment to gains in SFH precision from jointly fitting stellar metallicities and CMDs.« less
Research on the precision measurement of super-low reflectivity
NASA Astrophysics Data System (ADS)
Yuan, Hao-yu; Lu, Zong-gui; Xia, Yan-wen; Peng, Zhi-tao; Liu, Hua; Xu, Long-bo; Sun, Zhi-hong; Tang, Jun
2010-10-01
Introduced a high-precision measurement of measured the super-low reflectivity and small sampling angle. Using single reflect way measured, and compare with re-swatch. Testing the reflectance of the sampling mirror which be used on TIL, and analyze the error. Research results indicate, the main factor which affect result is energy detector error and energy detector linearity. This methods is easy and have high-precision, it can be used to measure the super-low reflectivity sampling mirror reflectance.
2008-12-01
Figure 2. Definition of Attitude Angles and Torque Components in Spacecraft Reference Frame...Figure 5. PD controller in ideal three-axis-stabilized spacecraft ADCS. ................................16 Figure 6. Extract Position Angles function in...performance of spacecraft systems. Two categories of system architectures are discussed: recursive data management, found in feedback control systems; and
NASA Technical Reports Server (NTRS)
Martin, Ken E.; Esztergalyos, J.
1992-01-01
The Bonneville Power Administration (BPA) uses IRIG-B transmitted over microwave as its primary system time dissemination. Problems with accuracy and reliability have led to ongoing research into better methods. BPA has also developed and deployed a unique fault locator which uses precise clocks synchronized by a pulse over microwaves. It automatically transmits the data to a central computer for analysis. A proposed system could combine fault location timing and time dissemination into a Global Position System (GPS) timing receiver and close the verification loop through a master station at the Dittmer Control Center. Such a system would have many advantages, including lower cost, higher reliability, and wider industry support. Test results indicate the GPS has sufficient accuracy and reliability for this and other current timing requirements including synchronous phase angle measurements. A phasor measurement system which provides phase angle has recently been tested with excellent results. Phase angle is a key parameter in power system control applications including dynamic braking, DC modulation, remedial action schemes, and system state estimation. Further research is required to determine the applications which can most effectively use real-time phase angle measurements and the best method to apply them.
NASA Astrophysics Data System (ADS)
Martin, Ken E.; Esztergalyos, J.
1992-07-01
The Bonneville Power Administration (BPA) uses IRIG-B transmitted over microwave as its primary system time dissemination. Problems with accuracy and reliability have led to ongoing research into better methods. BPA has also developed and deployed a unique fault locator which uses precise clocks synchronized by a pulse over microwaves. It automatically transmits the data to a central computer for analysis. A proposed system could combine fault location timing and time dissemination into a Global Position System (GPS) timing receiver and close the verification loop through a master station at the Dittmer Control Center. Such a system would have many advantages, including lower cost, higher reliability, and wider industry support. Test results indicate the GPS has sufficient accuracy and reliability for this and other current timing requirements including synchronous phase angle measurements. A phasor measurement system which provides phase angle has recently been tested with excellent results. Phase angle is a key parameter in power system control applications including dynamic braking, DC modulation, remedial action schemes, and system state estimation. Further research is required to determine the applications which can most effectively use real-time phase angle measurements and the best method to apply them.
Measurement method of rotation angle and clearance in intelligent spherical hinge
NASA Astrophysics Data System (ADS)
Hu, Penghao; Lu, Yichang; Chen, Shiyi; Hu, Yi; Zhu, Lianqing
2018-06-01
Precision ball hinges are widely applied in parallel mechanisms, robotics, and other areas, but their rotation orientation and angle cannot be obtained during passive motion. The simultaneous clearance error in a precision ball hinge’s motion also can not be determined. In this paper we propose an intelligent ball hinge (IBH) that can detect the rotation angle and moving clearance, based on our previous research results. The measurement model was optimized to promote measurement accuracy and resolution, and an optimal design for the IBH’s structure was determined. The experimental data showed that the measurement accuracy and resolution of the modified scheme were improved. Within ±10° and ± 20°, the average errors of the uniaxial measurements were 0.29° and 0.42°, respectively. The resolution of the measurements was 15″. The source of the measurement errors was analyzed through theory and experimental data and several key error sources were determined. A point capacitance model for measuring the clearance error is proposed, which is useful not only in compensating for the angle measurement error but also in realizing the motion clearance of an IBH in real-time.
A high precision dual feedback discrete control system designed for satellite trajectory simulator
NASA Astrophysics Data System (ADS)
Liu, Ximin; Liu, Liren; Sun, Jianfeng; Xu, Nan
2005-08-01
Cooperating with the free-space laser communication terminals, the satellite trajectory simulator is used to test the acquisition, pointing, tracking and communicating performances of the terminals. So the satellite trajectory simulator plays an important role in terminal ground test and verification. Using the double-prism, Sun etc in our group designed a satellite trajectory simulator. In this paper, a high precision dual feedback discrete control system designed for the simulator is given and a digital fabrication of the simulator is made correspondingly. In the dual feedback discrete control system, Proportional- Integral controller is used in velocity feedback loop and Proportional- Integral- Derivative controller is used in position feedback loop. In the controller design, simplex method is introduced and an improvement to the method is made. According to the transfer function of the control system in Z domain, the digital fabrication of the simulator is given when it is exposed to mechanism error and moment disturbance. Typically, when the mechanism error is 100urad, the residual standard error of pitching angle, azimuth angle, x-coordinate position and y-coordinate position are 0.49urad, 6.12urad, 4.56urad, 4.09urad respectively. When the moment disturbance is 0.1rad, the residual standard error of pitching angle, azimuth angle, x-coordinate position and y-coordinate position are 0.26urad, 0.22urad, 0.16urad, 0.15urad respectively. The digital fabrication results demonstrate that the dual feedback discrete control system designed for the simulator can achieve the anticipated high precision performance.
1999-07-25
This image of Neptune was taken through the clear filter of the narrow-angle camera on July 16, 1989 by NASA Voyager 2 spacecraft. The image was processed by computer to show the newly resolved dark oval feature embedded in the middle of the dusky south
Lü, Chun-guang; Wang, Wei-he; Yang, Wen-bo; Tian, Qing-iju; Lu, Shan; Chen, Yun
2015-11-01
New hyperspectral sensor to detect total ozone is considered to be carried on geostationary orbit platform in the future, because local troposphere ozone pollution and diurnal variation of ozone receive more and more attention. Sensors carried on geostationary satellites frequently obtain images on the condition of larger observation angles so that it has higher requirements of total ozone retrieval on these observation geometries. TOMS V8 algorithm is developing and widely used in low orbit ozone detecting sensors, but it still lack of accuracy on big observation geometry, therefore, how to improve the accuracy of total ozone retrieval is still an urgent problem that demands immediate solution. Using moderate resolution atmospheric transmission, MODT-RAN, synthetic UV backscatter radiance in the spectra region from 305 to 360 nm is simulated, which refers to clear sky, multi angles (12 solar zenith angles and view zenith angles) and 26 standard profiles, moreover, the correlation and trends between atmospheric total ozone and backward scattering of the earth UV radiation are analyzed based on the result data. According to these result data, a new modified initial total ozone estimation model in TOMS V8 algorithm is considered to be constructed in order to improve the initial total ozone estimating accuracy on big observation geometries. The analysis results about total ozone and simulated UV backscatter radiance shows: Radiance in 317.5 nm (R₃₁₇.₅) decreased as the total ozone rise. Under the small solar zenith Angle (SZA) and the same total ozone, R₃₁₇.₅ decreased with the increase of view zenith Angle (VZA) but increased on the large SZA. Comparison of two fit models shows: without the condition that both SZA and VZA are large (> 80°), exponential fitting model and logarithm fitting model all show high fitting precision (R² > 0.90), and precision of the two decreased as the SZA and VZA rise. In most cases, the precision of logarithm fitting mode is about 0.9% higher than exponential fitting model. With the increasing of VZA or SZA, the fitting precision gradually lower, and the fall is more in the larger VZA or SZA. In addition, the precision of fitting mode exist a plateau in the small SZA range. The modified initial total ozone estimating model (ln(I) vs. Ω) is established based on logarithm fitting mode, and compared with traditional estimating model (I vs. ln(Ω)), that shows: the RMSE of ln(I) vs. Ω and I vs. ln(Ω) all have the down trend with the rise of total ozone. In the low region of total ozone (175-275 DU), the RMSE is obvious higher than high region (425-525 DU), moreover, a RMSE peak and a trough exist in 225 and 475 DU respectively. With the increase of VZA and SZA, the RMSE of two initial estimating models are overall rise, and the upraising degree is ln(I) vs. Ω obvious with the growing of SZA and VZA. The estimating result by modified model is better than traditional model on the whole total ozone range (RMSE is 0.087%-0.537% lower than traditional model), especially on lower total ozone region and large observation geometries. Traditional estimating model relies on the precision of exponential fitting model, and modified estimating model relies on the precision of logarithm fitting model. The improvement of the estimation accuracy by modified initial total ozone estimating model expand the application range of TOMS V8 algorithm. For sensor carried on geostationary orbit platform, there is no doubt that the modified estimating model can help improve the inversion accuracy on wide spatial and time range This modified model could give support and reference to TOMS algorithm update in the future.
Wu, Pei-Hsin; Cheng, Cheng-Chieh; Wu, Ming-Long; Chao, Tzu-Cheng; Chung, Hsiao-Wen; Huang, Teng-Yi
2014-01-01
The dual echo steady-state (DESS) sequence has been shown successful in achieving fast T2 mapping with good precision. Under-estimation of T2, however, becomes increasingly prominent as the flip angle decreases. In 3D DESS imaging, therefore, the derived T2 values would become a function of the slice location in the presence of non-ideal slice profile of the excitation RF pulse. Furthermore, the pattern of slice-dependent variation in T2 estimates is dependent on the RF pulse waveform. Multi-slice 2D DESS imaging provides better inter-slice consistency, but the signal intensity is subject to integrated effects of within-slice distribution of the actual flip angle. Consequently, T2 measured using 2D DESS is prone to inaccuracy even at the designated flip angle of 90°. In this study, both phantom and human experiments demonstrate the above phenomena in good agreement with model prediction. © 2013.
Proposal for a trigonometric method to evaluate the abduction angle of the lower limbs in neonates.
Lima, Thaís; Alves, Cyntia; Funayama, Carolina A R
2008-12-01
It is difficult to precisely measure articular arc movement in newborns using a goniometer. This article proposes an objective method based on trigonometry for the evaluation of lower limb abduction. With the newborn aligned in the dorsal decubitus position, 2 points are marked at the level of the medial malleolus, one on the sagittal line and the other at the end of the abduction. Using the right-sided line between these 2 points and a line from the medial malleolus to the reference point at the anterior superior iliac spine or umbilical scar, an isosceles triangle is drawn, and half of the inferential abduction angle is obtained by calculating the sine. Twenty healthy full-term newborns comprise the study cohort. Intersubject and intrasubject variability among the abduction angle values (mean [SD], 37 degrees [4] degrees) is low. This method is advantageous because the measurement is precise and because the sine can be used without approximation.
Dong, Ling-Bo; Liu, Zhao-Gang; Li, Feng-Ri; Jiang, Li-Chun
2013-09-01
By using the branch analysis data of 955 standard branches from 60 sampled trees in 12 sampling plots of Pinus koraiensis plantation in Mengjiagang Forest Farm in Heilongjiang Province of Northeast China, and based on the linear mixed-effect model theory and methods, the models for predicting branch variables, including primary branch diameter, length, and angle, were developed. Considering tree effect, the MIXED module of SAS software was used to fit the prediction models. The results indicated that the fitting precision of the models could be improved by choosing appropriate random-effect parameters and variance-covariance structure. Then, the correlation structures including complex symmetry structure (CS), first-order autoregressive structure [AR(1)], and first-order autoregressive and moving average structure [ARMA(1,1)] were added to the optimal branch size mixed-effect model. The AR(1) improved the fitting precision of branch diameter and length mixed-effect model significantly, but all the three structures didn't improve the precision of branch angle mixed-effect model. In order to describe the heteroscedasticity during building mixed-effect model, the CF1 and CF2 functions were added to the branch mixed-effect model. CF1 function improved the fitting effect of branch angle mixed model significantly, whereas CF2 function improved the fitting effect of branch diameter and length mixed model significantly. Model validation confirmed that the mixed-effect model could improve the precision of prediction, as compare to the traditional regression model for the branch size prediction of Pinus koraiensis plantation.
della Croce, U; Cappozzo, A; Kerrigan, D C
1999-03-01
Human movement analysis using stereophotogrammetry is based on the reconstruction of the instantaneous laboratory position of selected bony anatomical landmarks (AL). For this purpose, knowledge of an AL's position in relevant bone-embedded frames is required. Because ALs are not points but relatively large and curved areas, their identification by palpation or other means is subject to both intra- and inter-examiner variability. In addition, the local position of ALs, as reconstructed using an ad hoc experimental procedure (AL calibration), is affected by photogrammetric errors. The intra- and inter-examiner precision with which local positions of pelvis and lower limb palpable bony ALs can be identified and reconstructed were experimentally assessed. Six examiners and two subjects participated in the study. Intra- and inter-examiner precision (RMS distance from the mean position) resulted in the range 6-21 mm and 13-25 mm, respectively. Propagation of the imprecision of ALs to the orientation of bone-embedded anatomical frames and to hip, knee and ankle joint angles was assessed. Results showed that this imprecision may cause distortion in joint angle against time functions to the extent that information relative to angular movements in the range of 10 degrees or lower may be concealed. Bone geometry parameters estimated using the same data showed that the relevant precision does not allow for reliable bone geometry description. These findings, together with those relative to skin movement artefacts reported elsewhere, assist the human movement analyst's consciousness of the possible limitations involved in 3D movement analysis using stereophotogrammetry and call for improvements of the relevant experimental protocols.
Study of multi-functional precision optical measuring system for large scale equipment
NASA Astrophysics Data System (ADS)
Jiang, Wei; Lao, Dabao; Zhou, Weihu; Zhang, Wenying; Jiang, Xingjian; Wang, Yongxi
2017-10-01
The effective application of high performance measurement technology can greatly improve the large-scale equipment manufacturing ability. Therefore, the geometric parameters measurement, such as size, attitude and position, requires the measurement system with high precision, multi-function, portability and other characteristics. However, the existing measuring instruments, such as laser tracker, total station, photogrammetry system, mostly has single function, station moving and other shortcomings. Laser tracker needs to work with cooperative target, but it can hardly meet the requirement of measurement in extreme environment. Total station is mainly used for outdoor surveying and mapping, it is hard to achieve the demand of accuracy in industrial measurement. Photogrammetry system can achieve a wide range of multi-point measurement, but the measuring range is limited and need to repeatedly move station. The paper presents a non-contact opto-electronic measuring instrument, not only it can work by scanning the measurement path but also measuring the cooperative target by tracking measurement. The system is based on some key technologies, such as absolute distance measurement, two-dimensional angle measurement, automatically target recognition and accurate aiming, precision control, assembly of complex mechanical system and multi-functional 3D visualization software. Among them, the absolute distance measurement module ensures measurement with high accuracy, and the twodimensional angle measuring module provides precision angle measurement. The system is suitable for the case of noncontact measurement of large-scale equipment, it can ensure the quality and performance of large-scale equipment throughout the process of manufacturing and improve the manufacturing ability of large-scale and high-end equipment.
Energy-resolved coherent diffraction from laser-driven electronic motion in atoms
NASA Astrophysics Data System (ADS)
Shao, Hua-Chieh; Starace, Anthony F.
2017-10-01
We investigate theoretically the use of energy-resolved ultrafast electron diffraction to image laser-driven electronic motion in atoms. A chirped laser pulse is used to transfer the valence electron of the lithium atom from the ground state to the first excited state. During this process, the electronic motion is imaged by 100-fs and 1-fs electron pulses in energy-resolved diffraction measurements. Simulations show that the angle-resolved spectra reveal the time evolution of the energy content and symmetry of the electronic state. The time-dependent diffraction patterns are further interpreted in terms of the momentum transfer. For the case of incident 1-fs electron pulses, the rapid 2 s -2 p quantum beat motion of the target electron is imaged as a time-dependent asymmetric oscillation of the diffraction pattern.
NASA Astrophysics Data System (ADS)
Yang, Bo; Wang, Dehui; Zhou, Lin; Wu, Shuang; Xiang, Rong; Zhang, Wenhua; Gui, Huaqiao; Liu, Jianguo; Wang, Huanqing; Lu, Liang; Yu, Benli
2017-06-01
The self-mixing technique based on the traditional reflecting mirror has been demonstrated with great merit for angle sensing applications. Here we demonstrate a modified self-reflection-mixing angle measurement system by combine a right-angle prism to self-mixing angle measurement. In our system, the wavelength is crucial to the angle measurement resolution. For a microchip solid-state laser, the measurement resolution can reach 0.49 mrad, while the resolution for the He-Ne laser is 0.53 mrad. In addition, the ranges in the system with the microchip solid-state laser and He-Ne laser are up to 22 mrad and 24.9 mrad respectively. This modified angle measurement system effectively combines the advantage of self-mixing measurement system with a compact structure, providing interesting features such as of high requisition of resolution and precision.
Navy Precision Optical Interferometer Measurements of 10 Stellar Oscillators
2014-02-01
and used photometry from the literature to calculate their bolometric fluxes, luminosities, and effective temperatures. We then used our results to test...oscillations that were bright enough to observing using the NPOI, which has a magnitude limit of V = 6.5. They also had to be resolved with the longest...calibrators are stars that are significantly less resolved on the baselines used than the targets. This meant that uncertainties in the calibrator’s
Search for CP violation effects in the h→ τ τ decay with e^+e^- colliders
NASA Astrophysics Data System (ADS)
Chen, Xin; Wu, Yongcheng
2017-10-01
A new method is proposed to reconstruct the neutrinos in the e^+e^-→ Zh process followed by the h→ τ τ decay. With the help of a refined Higgs momentum reconstruction from the recoiling system and the impact parameters, high precision in the determination of the momentum of neutrinos can be achieved. The prospect of measuring the Higgs CP mixing angle with the h→ τ τ decay at e^+e^- colliders is studied with the new method. The analysis is based on a detailed detector simulation of the signal and backgrounds. The fully reconstructed neutrinos and also other visible products from the tau decay are used to build matrix element (ME)-based CP observables. With 5 ab^{-1} of data at E_{ {CM}}=250 GeV, a precision of 2.9° can be achieved for the CP mixing angle with three main one-prong decay modes of the taus. The precision is found to be about 35% better than the other methods.
Ho, Derek; Drake, Tyler K; Smith-McCune, Karen K; Darragh, Teresa M; Hwang, Loris Y; Wax, Adam
2017-03-15
This study sought to establish the feasibility of using in situ depth-resolved nuclear morphology measurements for detection of cervical dysplasia. Forty enrolled patients received routine cervical colposcopy with angle-resolved low coherence interferometry (a/LCI) measurements of nuclear morphology. a/LCI scans from 63 tissue sites were compared to histopathological analysis of co-registered biopsy specimens which were classified as benign, low-grade squamous intraepithelial lesion (LSIL), or high-grade squamous intraepithelial lesion (HSIL). Results were dichotomized as dysplastic (LSIL/HSIL) versus non-dysplastic and HSIL versus LSIL/benign to determine both accuracy and potential clinical utility of a/LCI nuclear morphology measurements. Analysis of a/LCI data was conducted using both traditional Mie theory based processing and a new hybrid algorithm that provides improved processing speed to ascertain the feasibility of real-time measurements. Analysis of depth-resolved nuclear morphology data revealed a/LCI was able to detect a significant increase in the nuclear diameter at the depth bin containing the basal layer of the epithelium for dysplastic versus non-dysplastic and HSIL versus LSIL/Benign biopsy sites (both p < 0.001). Both processing techniques resulted in high sensitivity and specificity (>0.80) in identifying dysplastic biopsies and HSIL. The hybrid algorithm demonstrated a threefold decrease in processing time at a slight cost in classification accuracy. The results demonstrate the feasibility of using a/LCI as an adjunctive clinical tool for detecting cervical dysplasia and guiding the identification of optimal biopsy sites. The faster speed from the hybrid algorithm offers a promising approach for real-time clinical analysis. © 2016 UICC.
Ho, Derek; Drake, Tyler K.; Smith-McCune, Karen K.; Darragh, Teresa M.; Hwang, Loris Y.; Wax, Adam
2017-01-01
This study sought to establish the feasibility of using in situ depth-resolved nuclear morphology measurements for detection of cervical dysplasia. Forty (40) enrolled patients received routine cervical colposcopy with angle-resolved low coherence interferometry (a/LCI) measurements of nuclear morphology. a/LCI scans from 63 tissue sites were compared to histopathological analysis of co-registered biopsy specimens which were classified as benign, low-grade squamous intraepithelial lesion (LSIL), or high-grade squamous intraepithelial lesion (HSIL). Results were dichotomized as dysplastic (LSIL/HSIL) versus non-dysplastic and HSIL versus LSIL/benign to determine both accuracy and potential clinical utility of a/LCI nuclear morphology measurements. Analysis of a/LCI data was conducted using both traditional Mie theory based processing and a new hybrid algorithm that provides improved processing speed to ascertain the feasibility of real-time measurements. Analysis of depth-resolved nuclear morphology data revealed a/LCI was able to detect a significant increase in the nuclear diameter at the depth bin containing the basal layer of the epithelium for dysplastic versus non-dysplastic and HSIL versus LSIL/Benign biopsy sites (both p < 0.001). Both processing techniques resulted in high sensitivity and specificity (> 0.80) in identifying dysplastic biopsies and HSIL. The hybrid algorithm demonstrated a threefold decrease in processing time at a slight cost in classification accuracy. The results demonstrate the feasibility of using a/LCI as an adjunctive clinical tool for detecting cervical dysplasia and guiding the identification of optimal biopsy sites. The faster speed from the hybrid algorithm offers a promising approach for real-time clinical analysis. PMID:27883177
NASA Astrophysics Data System (ADS)
Zhou, Zengxiang; Jin, Yi; Zhai, Chao; Xing, Xiaozheng
2008-07-01
In the LAMOST project, the unit-holes on the Focal Plane Plate are the final installation location of the optical fiber positioning system. Theirs precision will influence the observation efficiency of the LAMOST. For the unique requirements, the unit-holes on the Focal Plane Plate are composed by a series of tiny angle dimensional holes which dimensional angle are between 16' to 2.5°. According to these requirements, the measurement of the tiny angle dimensional holes for the unit-holes needs to less than 3'. And all the unit-holes point to the virtual sphere center of the Focal Plane Plate. To that end, the angle departure of the unit-holes axis is changed to the distance from the virtual sphere center of Focal Plane Plate to the unit-holes axis. That is the better way to evaluate the technical requirements of the dimensional angle errors. In the measuring process, common measuring methods do not fit for the tiny angle dimensional hole by CMM(coordinate measurement machine). An extraordinary way to solve this problem is to insert a measuring stick into a unit-hole, with a target ball on the stick. Then measure the low point of the ball center and pull out the stick for the high station of center. Finally, calculate the two points for the unit-hole axis to get the angle departure. But on the other hand, use this methods will bring extra errors for the measuring stick and the target ball. For better analysis this question, a series experiments are mentioned in this paper, which testify that the influence of the measure implement is little. With increasing the distance between the low point and the high point position in the measuring process should enhance the accuracy of dimensional angle measurement.
Zawadzki, Robert J; Zhang, Pengfei; Zam, Azhar; Miller, Eric B; Goswami, Mayank; Wang, Xinlei; Jonnal, Ravi S; Lee, Sang-Hyuck; Kim, Dae Yu; Flannery, John G; Werner, John S; Burns, Marie E; Pugh, Edward N
2015-06-01
Adaptive optics scanning laser ophthalmoscopy (AO-SLO) has recently been used to achieve exquisite subcellular resolution imaging of the mouse retina. Wavefront sensing-based AO typically restricts the field of view to a few degrees of visual angle. As a consequence the relationship between AO-SLO data and larger scale retinal structures and cellular patterns can be difficult to assess. The retinal vasculature affords a large-scale 3D map on which cells and structures can be located during in vivo imaging. Phase-variance OCT (pv-OCT) can efficiently image the vasculature with near-infrared light in a label-free manner, allowing 3D vascular reconstruction with high precision. We combined widefield pv-OCT and SLO imaging with AO-SLO reflection and fluorescence imaging to localize two types of fluorescent cells within the retinal layers: GFP-expressing microglia, the resident macrophages of the retina, and GFP-expressing cone photoreceptor cells. We describe in detail a reflective afocal AO-SLO retinal imaging system designed for high resolution retinal imaging in mice. The optical performance of this instrument is compared to other state-of-the-art AO-based mouse retinal imaging systems. The spatial and temporal resolution of the new AO instrumentation was characterized with angiography of retinal capillaries, including blood-flow velocity analysis. Depth-resolved AO-SLO fluorescent images of microglia and cone photoreceptors are visualized in parallel with 469 nm and 663 nm reflectance images of the microvasculature and other structures. Additional applications of the new instrumentation are discussed.
Total photoionization cross sections of atomic oxygen from threshold to 44.3 A
NASA Technical Reports Server (NTRS)
Angel, G. C.; Samson, James A. R.
1988-01-01
Synchrotron radiation was used to obtain the relative photoionization cross section of atomic oxygen for the production of singly charged ions over the 44.3-910.5-A wavelength range. Measurement of the contribution of multiple ionization to the cross sections has made possible the determination of total photoionization cross sections below 250 A. The series of autoionizing resonances leading to the 4P state of the oxygen ion has been observed using an ionization-type experimental procedure for the first time.
Effects of configuration interaction on photoabsorption spectra in the continuum
NASA Astrophysics Data System (ADS)
Komninos, Yannis; Nicolaides, Cleanthes A.
2004-10-01
It is pointed out that the proper interpretation of a recently published experimental spectrum from the multilaser photoionization of Sr [Eichmann , Phys. Rev. Lett. 90, 233004 (2003)] must account for a radiative transition between two autoionizing states. The application of orthonormality selection rules and of configuration-interaction theory involving the continuous spectrum and the quasicontinuum of the upper part of Rydberg series explains quantitatively the appearance, the shape, and the variation of heights of the observed peaks of resonances.
Ab initio studies of dissociative recombination
NASA Technical Reports Server (NTRS)
Guberman, Steven L.
1989-01-01
Quantum chemical calculations of the dissociative recombination of O2(+) and N2(+) are reported. An approach for calculating autoionization widths from high-principal-quantum-number Rydberg states is summarized, and an example is presented for the lowest dissociative state of O2. For O2(+), the 1Sigma(+)u state is the sole source of O(1S) from the lowest 10 vibrational levels of the ion. Rate coefficients for generating O(1S) and O(1D) at ionospheric temperatures are reported.
NASA Astrophysics Data System (ADS)
Deshmukh, Pranawa C.; Johnson, W. R.
1983-01-01
A study of the photoionization of calcium in the relativistic random-phase approximation is reported. Predictions of photoionization cross sections, angular distribution asymmetry parameters, and spin-polarization parameters for the 4s, 3p, and 3s subshells are made with emphasis on the energy region above the 3p32 threshold where multiconfigurational effects are not expected to be very important. Autoionization resonances below the 3s threshold and between the 3p32 and 3p12 thresholds are analyzed using the relativistic multichannel quantum-defect theory.
High-Precision Half-Life Measurements for the Superallowed Fermi β+ Emitters 14O and 18Ne
NASA Astrophysics Data System (ADS)
Laffoley, A. T.; Andreoiu, C.; Austin, R. A. E.; Ball, G. C.; Bender, P. C.; Bidaman, H.; Bildstein, V.; Blank, B.; Bouzomita, H.; Cross, D. S.; Deng, G.; Diaz Varela, A.; Dunlop, M. R.; Dunlop, R.; Finlay, P.; Garnsworthy, A. B.; Garrett, P.; Giovinazzo, J.; Grinyer, G. F.; Grinyer, J.; Hadinia, B.; Jamieson, D. S.; Jigmeddorj, B.; Ketelhut, S.; Kisliuk, D.; Leach, K. G.; Leslie, J. R.; MacLean, A.; Miller, D.; Mills, B.; Moukaddam, M.; Radich, A. J.; Rajabali, M. M.; Rand, E. T.; Svensson, C. E.; Tardiff, E.; Thomas, J. C.; Turko, J.; Voss, P.; Unsworth, C.
High-precision half-life measurements, at the level of ±0.04%, for the superallowed Fermi emitters 14O and 18Ne have been performed at TRIUMF's Isotope Separator and Accelerator facility. Using 3 independent detector systems, a gas-proportional counter, a fast plastic scintillator, and a high-purity germanium array, a series of direct β and γ counting measurements were performed for each of the isotopes. In the case of 14O, these measurements were made to help resolve an existing discrepancy between detection methods, whereas for 18Ne the half-life precision has been improved in anticipation of forthcoming high-precision branching ratio measurements.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Su, L. N.; Hu, Z. D.; Zheng, Y.
2014-09-15
Proton acceleration from 4 μm thick aluminum foils irradiated by 30-TW Ti:sapphire laser pulses is investigated using an angle-resolved proton energy spectrometer. We find that a modulated spectral peak at ∼0.82 MeV is presented at 2.5° off the target normal direction. The divergence angle of the modulated zone is 3.8°. Two-dimensional particle-in-cell simulations reveal that self-generated toroidal magnetic field at the rear surface of the target foil is responsible for the modulated spectral feature. The field deflects the low energy protons, resulting in the modulated energy spectrum with certain peaks.
Comparison of intersecting pedestrian flows based on experiments
NASA Astrophysics Data System (ADS)
Zhang, J.; Seyfried, A.
2014-07-01
Intersections of pedestrian flows feature multiple types, varying in the numbers of flow directions as well as intersecting angles. In this article results from intersecting flow experiments with two different intersecting angles are compared. To analyze the transport capabilities the Voronoi method is used to resolve the fine structure of the resulting velocity-density relations and spatial dependence of the measurements. The fundamental diagrams of various flow types are compared and show no apparent difference with respect to the intersecting angle 90° and 180°. This result indicates that head-on conflicts of different types of flow have the same influence on the transport properties of the system, which demonstrates the high self-organization capabilities of pedestrians.
One-dimensional pinning behavior in Co-doped BaFe2As2 thin films
NASA Astrophysics Data System (ADS)
Mishev, V.; Seeböck, W.; Eisterer, M.; Iida, K.; Kurth, F.; Hänisch, J.; Reich, E.; Holzapfel, B.
2013-12-01
Angle-resolved transport measurements revealed that planar defects dominate flux pinning in the investigated Co-doped BaFe2As2 thin film. For any given field and temperature, the critical current depends only on the angle between the crystallographic c-axis and the applied magnetic field but not on the angle between the current and the field. The critical current is therefore limited only by the in-plane component of the Lorentz force but independent of the out-of-plane component, which is entirely balanced by the pinning force exerted by the planar defects. This one-dimensional pinning behavior shows similarities and differences to intrinsic pinning in layered superconductors.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Just, J.; Lützenkirchen-Hecht, D.; Müller, O.
The depth distribution of secondary phases in the solar cell absorber material Cu 2ZnSnS 4 (CZTS) is quantitatively investigated using X-ray Absorption Near Edge Structure (XANES) analysis at the K-edge of sulfur at varying incidence angles. Varying information depths from several nanometers up to the full thickness is achieved. A quantitative profile of the phase distribution is obtained by a self-consistent fit of a multilayer model to the XANES spectra for different angles. Single step co-evaporated CZTS thin-films are found to exhibit zinc and copper sulfide secondary phases preferentially at the front or back interfaces of the film.
Just, J.; Lützenkirchen-Hecht, D.; Müller, O.; ...
2017-12-12
The depth distribution of secondary phases in the solar cell absorber material Cu 2ZnSnS 4 (CZTS) is quantitatively investigated using X-ray Absorption Near Edge Structure (XANES) analysis at the K-edge of sulfur at varying incidence angles. Varying information depths from several nanometers up to the full thickness is achieved. A quantitative profile of the phase distribution is obtained by a self-consistent fit of a multilayer model to the XANES spectra for different angles. Single step co-evaporated CZTS thin-films are found to exhibit zinc and copper sulfide secondary phases preferentially at the front or back interfaces of the film.
Annually resolved atmospheric radiocarbon records reconstructed from tree-rings
NASA Astrophysics Data System (ADS)
Wacker, Lukas; Bleicher, Niels; Büntgen, Ulf; Friedrich, Michael; Friedrich, Ronny; Diego Galván, Juan; Hajdas, Irka; Jull, Anthony John; Kromer, Bernd; Miyake, Fusa; Nievergelt, Daniel; Reinig, Frederick; Sookdeo, Adam; Synal, Hans-Arno; Tegel, Willy; Wesphal, Torsten
2017-04-01
The IntCal13 calibration curve is mainly based on data measured by decay counting with a resolution of 10 years. Thus high frequency changes like the 11-year solar cycles or cosmic ray events [1] are not visible, or at least not to their full extent. New accelerator mass spectrometry (AMS) systems today are capable of measuring at least as precisely as decay counters [2], with the advantage of using 1000 times less material. The low amount of material required enables more efficient sample preparation. Thus, an annually resolved re-measurement of the tree-ring based calibration curve can now be envisioned. We will demonstrate with several examples the multitude of benefits resulting from annually resolved radiocarbon records from tree-rings. They will not only allow for more precise radiocarbon dating but also contain valuable new astrophysical information. The examples shown will additionally indicate that it can be critical to compare AMS measurements with a calibration curve that is mainly based on decay counting. We often see small offsets between the two measurement techniques, while the reason is yet unknown. [1] Miyake F, Nagaya K, Masuda K, Nakamura T. 2012. A signature of cosmic-ray increase in AD 774-775 from tree rings in Japan. Nature 486(7402):240-2. [2] Wacker L, Bonani G, Friedrich M, Hajdas I, Kromer B, Nemec M, Ruff M, Suter M, Synal H-A, Vockenhuber C. 2010. MICADAS: Routine and high-precision radiocarbon dating. Radiocarbon 52(2):252-62.
Element-resolved Kikuchi pattern measurements of non-centrosymmetric materials
DOE Office of Scientific and Technical Information (OSTI.GOV)
Vos, Maarten, E-mail: maarten.vos@anu.edu.au
2017-01-15
Angle-resolved electron Rutherford backscattering (ERBS) measurements using an electrostatic electron energy analyser can provide unique access to element-resolved crystallographic information. We present Kikuchi pattern measurements of the non-centrosymmetric crystal GaP, separately resolving the contributions of electrons backscattered from Ga and P. In comparison to element-integrated measurements like in the method of electron backscatter diffraction (EBSD), the effect of the absence of a proper 4-fold rotation axis in the point group of GaP can be sensed with a much higher visibility via the element-resolved Ga to P intensity ratio. These element-resolved measurements make it possible to experimentally attribute the previously observedmore » point-group dependent effect in element-integrated EBSD measurements to the larger contribution of electrons scattered from Ga compared to P. - Highlights: •Element specific Kikuchi patterns are presented for GaP. •Absence of a proper four-fold rotation axis is demonstrated. •Ga and P intensity variations after 90 degree rotation have opposite phase. •The asymmetry in the total intensity distribution resembles that of Ga.« less
Sensor-less pseudo-sinusoidal drive for a permanent-magnet brushless ac motor
NASA Astrophysics Data System (ADS)
Liu, Li-Hsiang; Chern, Tzuen-Lih; Pan, Ping-Lung; Huang, Tsung-Mou; Tsay, Der-Min; Kuang, Jao-Hwa
2012-04-01
The precise rotor-position information is required for a permanent-magnet brushless ac motor (BLACM) drive. In the conventional sinusoidal drive method, either an encoder or a resolver is usually employed. For position sensor-less vector control schemes, the rotor flux estimation and torque components are obtained by complicated coordinate transformations. These computational intensive methods are susceptible to current distortions and parameter variations. To simplify the method complexity, this work presents a sensor-less pseudo-sinusoidal drive scheme with speed control for a three-phase BLACM. Based on the sinusoidal drive scheme, a floating period of each phase current is inserted for back electromotive force detection. The zero-crossing point is determined directly by the proposed scheme, and the rotor magnetic position and rotor speed can be estimated simultaneously. Several experiments for various active angle periods are undertaken. Furthermore, a current feedback control is included to minimize and compensate the torque fluctuation. The experimental results show that the proposed method has a competitive performance compared with the conventional drive manners for BLACM. The proposed scheme is straightforward, bringing the benefits of sensor-less drive and negating the need for coordinate transformations in the operating process.
Wavefront detection method of a single-sensor based adaptive optics system.
Wang, Chongchong; Hu, Lifa; Xu, Huanyu; Wang, Yukun; Li, Dayu; Wang, Shaoxin; Mu, Quanquan; Yang, Chengliang; Cao, Zhaoliang; Lu, Xinghai; Xuan, Li
2015-08-10
In adaptive optics system (AOS) for optical telescopes, the reported wavefront sensing strategy consists of two parts: a specific sensor for tip-tilt (TT) detection and another wavefront sensor for other distortions detection. Thus, a part of incident light has to be used for TT detection, which decreases the light energy used by wavefront sensor and eventually reduces the precision of wavefront correction. In this paper, a single Shack-Hartmann wavefront sensor based wavefront measurement method is presented for both large amplitude TT and other distortions' measurement. Experiments were performed for testing the presented wavefront method and validating the wavefront detection and correction ability of the single-sensor based AOS. With adaptive correction, the root-mean-square of residual TT was less than 0.2 λ, and a clear image was obtained in the lab. Equipped on a 1.23-meter optical telescope, the binary stars with angle distance of 0.6″ were clearly resolved using the AOS. This wavefront measurement method removes the separate TT sensor, which not only simplifies the AOS but also saves light energy for subsequent wavefront sensing and imaging, and eventually improves the detection and imaging capability of the AOS.
Spectroscopic evidence for a type II Weyl semimetallic state in MoTe 2
Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki; ...
2016-07-11
In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential μ is tuned precisely to the Dirac/Weyl point. Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap. This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. Here we present the discovery of a type II topological Weyl semimetal state in pure MoTe 2, where two sets of Weyl points ( W±2 , W±3) existmore » at the touching points of electron and hole pockets and are located at different binding energies above E F. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface ‘track states’ that form closed loops and are unique to type II Weyl semimetals. Lastly, this material provides an exciting, new platform to study the properties of Weyl fermions.« less
Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2
NASA Astrophysics Data System (ADS)
Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki; Zhao, Zhiying; Suzuki, Michi-To; Arita, Ryotaro; Wu, Yun; Mou, Daixiang; Cao, Huibo; Yan, Jiaqiang; Trivedi, Nandini; Kaminski, Adam
2016-11-01
In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential μ is tuned precisely to the Dirac/Weyl point. Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap. This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. Here we present the discovery of a type II topological Weyl semimetal state in pure MoTe2, where two sets of Weyl points (, ) exist at the touching points of electron and hole pockets and are located at different binding energies above EF. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface `track states' that form closed loops and are unique to type II Weyl semimetals. This material provides an exciting, new platform to study the properties of Weyl fermions.
Neutze, Richard
2014-07-17
X-ray free-electron lasers (XFELs) are revolutionary X-ray sources. Their time structure, providing X-ray pulses of a few tens of femtoseconds in duration; and their extreme peak brilliance, delivering approximately 10(12) X-ray photons per pulse and facilitating sub-micrometre focusing, distinguish XFEL sources from synchrotron radiation. In this opinion piece, I argue that these properties of XFEL radiation will facilitate new discoveries in life science. I reason that time-resolved serial femtosecond crystallography and time-resolved wide angle X-ray scattering are promising areas of scientific investigation that will be advanced by XFEL capabilities, allowing new scientific questions to be addressed that are not accessible using established methods at storage ring facilities. These questions include visualizing ultrafast protein structural dynamics on the femtosecond to picosecond time-scale, as well as time-resolved diffraction studies of non-cyclic reactions. I argue that these emerging opportunities will stimulate a renaissance of interest in time-resolved structural biochemistry.
Resolving runaway electron distributions in space, time, and energy
Paz-Soldan, Carlos; Cooper, C. M.; Aleynikov, P.; ...
2018-05-01
Areas of agreement and disagreement with present-day models of RE evolution are revealed by measuring MeV-level bremsstrahlung radiation from runaway electrons (REs) with a pinhole camera. Spatially-resolved measurements localize the RE beam, reveal energy-dependent RE transport, and can be used to perform full two-dimensional (energy and pitch-angle) inversions of the RE phase space distribution. Energy-resolved measurements find qualitative agreement with modeling on the role of collisional and synchrotron damping in modifying the RE distribution shape. Measurements are consistent with predictions of phase-space attractors that accumulate REs, with non-monotonic features observed in the distribution. Temporally-resolved measurements find qualitative agreement with modelingmore » on the impact of collisional and synchrotron damping in varying the RE growth and decay rate. Anomalous RE loss is observed and found to be largest at low energy. As a result, possible roles for kinetic instability or spatial transport to resolve these anomalies are discussed.« less
Resolving runaway electron distributions in space, time, and energy
DOE Office of Scientific and Technical Information (OSTI.GOV)
Paz-Soldan, Carlos; Cooper, C. M.; Aleynikov, P.
Areas of agreement and disagreement with present-day models of RE evolution are revealed by measuring MeV-level bremsstrahlung radiation from runaway electrons (REs) with a pinhole camera. Spatially-resolved measurements localize the RE beam, reveal energy-dependent RE transport, and can be used to perform full two-dimensional (energy and pitch-angle) inversions of the RE phase space distribution. Energy-resolved measurements find qualitative agreement with modeling on the role of collisional and synchrotron damping in modifying the RE distribution shape. Measurements are consistent with predictions of phase-space attractors that accumulate REs, with non-monotonic features observed in the distribution. Temporally-resolved measurements find qualitative agreement with modelingmore » on the impact of collisional and synchrotron damping in varying the RE growth and decay rate. Anomalous RE loss is observed and found to be largest at low energy. As a result, possible roles for kinetic instability or spatial transport to resolve these anomalies are discussed.« less
NASA Astrophysics Data System (ADS)
Shelly, D. R.; Ellsworth, W. L.; Prejean, S. G.; Hill, D. P.; Hardebeck, J.; Hsieh, P. A.
2015-12-01
Earthquake swarms, sequences of sustained seismicity, convey active subsurface processes that sometimes precede larger tectonic or volcanic episodes. Their extended activity and spatiotemporal migration can often be attributed to fluid pressure transients as migrating crustal fluids (typically water and CO2) interact with subsurface structures. Although the swarms analyzed here are interpreted to be natural in origin, the mechanisms of seismic activation likely mirror those observed for earthquakes induced by industrial fluid injection. Here, we use massive-scale waveform correlation to detect and precisely locate 3-10 times as many earthquakes as included in routine catalogs for recent (2014-2015) swarms beneath Mammoth Mountain, Long Valley Caldera, Lassen Volcanic Center, and Fillmore areas of California, USA. These enhanced catalogs, with location precision as good as a few meters, reveal signatures of fluid-faulting interactions, such as systematic migration, fault-valve behavior, and fracture mesh structures, not resolved in routine catalogs. We extend this analysis to characterize source mechanism similarity even for very small newly detected events using relative P and S polarity estimates. This information complements precise locations to define fault complexities that would otherwise be invisible. In particular, although swarms often consist of groups of highly similar events, some swarms contain a population of outliers with different slip and/or fault orientations. These events highlight the complexity of fluid-faulting interactions. Despite their different settings, the four swarms analyzed here share many similarities, including pronounced hypocenter migration suggestive of a fluid pressure trigger. This includes the July 2015 Fillmore swarm, which, unlike the others, occurred outside of an obvious volcanic zone. Nevertheless, it exhibited systematic westward and downdip migration on a ~1x1.5 km low-angle, NW-dipping reverse fault at midcrustal depth.
An Externally Dispersed Interferometer for Sensitive Doppler Extrasolar Planet Searches
NASA Astrophysics Data System (ADS)
Ge, Jian; Erskine, David J.; Rushford, Mike
2002-09-01
A new kind of instrument for sensitive Doppler extrasolar planet searches, called an externally dispersed interferometer, is described in this paper. It is a combination of an optical Michelson-type interferometer and an intermediate-resolution grating spectrometer. The interferometer measures Doppler radial velocity (RV) variations of starlight through the phase shifts of moiré fringes, created by multiplication of the interferometer fringes with stellar absorption lines. The intermediate-resolution spectrograph disperses the moiré fringes into thousands of parallel-wavelength channels. This increases the instrument bandwidth and fringe visibility by preventing fringe cross-talk between neighboring spectral lines. This results in a net increase in the signal-to-noise ratio over an interferometer used alone with broadband light. Compared to current echelle spectrometers for extrasolar planet searches, this instrument offers two unique instrument properties: a simple, stable, well-defined sinusoidal instrument response function (point-spread function) and magnification of Doppler motion through moiré fringe techniques. Since instrument noise is chiefly limited by the ability to characterize the instrument response, this new technique provides unprecedented low instrumental noise in an economical compact apparatus, enabling higher precision for Doppler RV measurements. In practice, the moiré magnification can be 5-10 times depending on the interferometer comb angle. This instrument has better sensitivity for smaller Doppler shifts than echelle spectrometers. The instrument can be designed with much lower spectral resolving power without losing Doppler sensitivity and optimized for higher throughput than echelle spectrometers to allow a potential survey for planets around fainter stars than current magnitude limits. Lab-based experiments with a prototype instrument with a spectral resolution of R~20,000 demonstrated ~0.7 m s-1 precision for short-term RV measurements. A fiber-fed version of the prototype with R~5600 was tested with starlight at the Lick 1 m telescope and demonstrated ~7 m s-1 RV precision at 340 Å bandwidth. The increased velocity noise is attributed to the lower spectral resolution, lower fringe visibility, and uncontrolled instrument environment.
Achieving sub-millimetre precision with a solid-state full-field heterodyning range imaging camera
NASA Astrophysics Data System (ADS)
Dorrington, A. A.; Cree, M. J.; Payne, A. D.; Conroy, R. M.; Carnegie, D. A.
2007-09-01
We have developed a full-field solid-state range imaging system capable of capturing range and intensity data simultaneously for every pixel in a scene with sub-millimetre range precision. The system is based on indirect time-of-flight measurements by heterodyning intensity-modulated illumination with a gain modulation intensified digital video camera. Sub-millimetre precision to beyond 5 m and 2 mm precision out to 12 m has been achieved. In this paper, we describe the new sub-millimetre class range imaging system in detail, and review the important aspects that have been instrumental in achieving high precision ranging. We also present the results of performance characterization experiments and a method of resolving the range ambiguity problem associated with homodyne and heterodyne ranging systems.
Precision determination of electron scattering angle by differential nuclear recoil energy method
DOE Office of Scientific and Technical Information (OSTI.GOV)
Liyanage, N.; Saenboonruang, K.
2015-12-01
The accurate determination of the scattered electron angle is crucial to electron scattering experiments, both with open-geometry large-acceptance spectrometers and ones with dipole-type magnetic spectrometers for electron detection. In particular, for small central-angle experiments using dipole-type magnetic spectrometers, in which surveys are used to measure the spectrometer angle with respect to the primary electron beam, the importance of the scattering angle determination is emphasized. However, given the complexities of large experiments and spectrometers, the accuracy of such surveys is limited and insufficient to meet demands of some experiments. In this article, we present a new technique for determination of themore » electron scattering angle based on an accurate measurement of the primary beam energy and the principle of differential nuclear recoil. This technique was used to determine the scattering angle for several experiments carried out at the Experimental Hall A, Jefferson Lab. Results have shown that the new technique greatly improved the accuracy of the angle determination compared to surveys.« less
Precision Determination of Electron Scattering Angle by Differential Nuclear Recoil Energy Method
DOE Office of Scientific and Technical Information (OSTI.GOV)
Liyanage, Nilanga; Saenboonruang, Kiadtisak
2015-09-01
The accurate determination of the scattered electron angle is crucial to electron scattering experiments, both with open-geometry large-acceptance spectrometers and ones with dipole-type magnetic spectrometers for electron detection. In particular, for small central-angle experiments using dipole-type magnetic spectrometers, in which surveys are used to measure the spectrometer angle with respect to the primary electron beam, the importance of the scattering angle determination is emphasized. However, given the complexities of large experiments and spectrometers, the accuracy of such surveys is limited and insufficient to meet demands of some experiments. In this article, we present a new technique for determination of themore » electron scattering angle based on an accurate measurement of the primary beam energy and the principle of differential nuclear recoil. This technique was used to determine the scattering angle for several experiments carried out at the Experimental Hall A, Jefferson Lab. Results have shown that the new technique greatly improved the accuracy of the angle determination compared to surveys.« less
DOE Office of Scientific and Technical Information (OSTI.GOV)
Nishida, Jun; Fayer, Michael D., E-mail: fayer@stanford.edu
Functionalized organic monolayers deposited on planar two-dimensional surfaces are important systems for studying ultrafast orientational motions and structures of interfacial molecules. Several studies have successfully observed the orientational relaxation of functionalized monolayers by fluorescence depolarization experiments and recently by polarization-resolved heterodyne detected vibrational transient grating (HDTG) experiments. In this article we provide a model-independent theory to extract orientational correlation functions unique to interfacial molecules and other uniaxial systems based on polarization-resolved resonant third-order spectroscopies, such as pump-probe spectroscopy, HDTG spectroscopy, and fluorescence depolarization experiment. It will be shown (in the small beam-crossing angle limit) that five measurements are necessary tomore » completely characterize the monolayer's motions: I{sub ∥}(t) and I{sub ⊥}(t) with the incident beams normal to the surface, I{sub ∥}(t) and I{sub ⊥}(t) with a non-zero incident angle, and a time averaged linear dichroism measurement. Once these measurements are performed, two orientational correlation functions corresponding to in-plane and out-of-plane motions are obtained. The procedure is applicable not only for monolayers on flat surfaces, but any samples with uniaxial symmetry such as uniaxial liquid crystals and aligned planar bilayers. The theory is valid regardless of the nature of the actual molecular motions on interface. We then apply the general results to wobbling-in-a-cone model, in which molecular motions are restricted to a limited range of angles. Within the context of the model, the cone angle, the tilt of the cone relative to the surface normal, and the orientational diffusion constant can be determined. The results are extended to describe analysis of experiments where the beams are not crossing in the small angle limit.« less
NASA Astrophysics Data System (ADS)
Das, Saurish; Patel, H. V.; Milacic, E.; Deen, N. G.; Kuipers, J. A. M.
2018-01-01
We investigate the dynamics of a liquid droplet in contact with a surface of a porous structure by means of the pore-scale level, fully resolved numerical simulations. The geometrical details of the solid porous matrix are resolved by a sharp interface immersed boundary method on a Cartesian computational grid, whereas the motion of the gas-liquid interface is tracked by a mass conservative volume of fluid method. The numerical simulations are performed considering a model porous structure that is approximated by a 3D cubical scaffold with cylindrical struts. The effect of the porosity and the equilibrium contact angle (between the gas-liquid interface and the solid struts) on the spreading behavior, liquid imbibition, and apparent contact angle (between the gas-liquid interface and the porous base) are studied. We also perform several simulations for droplet spreading on a flat surface as a reference case. Gas-liquid systems of the Laplace number, La = 45 and La = 144 × 103 are considered neglecting the effect of gravity. We report the time exponent (n) and pre-factor (C) of the power law describing the evolution of the spreading diameter (S = Ctn) for different equilibrium contact angles and porosity. Our simulations reveal that the apparent or macroscopic contact angle varies linearly with the equilibrium contact angle and increases with porosity. Not necessarily for all the wetting porous structures, a continuous capillary drainage occurs, and we find that the rate of the capillary drainage very much depends on the fluid inertia. At La = 144 × 103, numerically we capture the capillary wave induced pinch-off and daughter droplet ejection. We observe that on the porous structure the pinch-off is weak compared to that on a flat plate.
A portable device for calibration of autocollimators with nanoradian precision
NASA Astrophysics Data System (ADS)
Yandayan, Tanfer
2017-09-01
A portable device has been developed in TUBITAK UME to calibrate high precision autocollimators with nanoradian precision. The device can operate in the range of +/-4500" which is far enough for the calibration of the available autocollimators and can generate ultra-small angles in measurement steps of 0.0005" (2.5 nrad). Description of the device with the performance tests using the calibrated precise autocollimators and novel methods will be reported. The test results indicate that the device is a good candidate for application to on-site/in-situ calibration of autocollimators with expanded uncertainties of 0.01" (50 nrad) particularly those used in slope measuring profilers.
Maximizing the Biochemical Resolving Power of Fluorescence Microscopy
Esposito, Alessandro; Popleteeva, Marina; Venkitaraman, Ashok R.
2013-01-01
Most recent advances in fluorescence microscopy have focused on achieving spatial resolutions below the diffraction limit. However, the inherent capability of fluorescence microscopy to non-invasively resolve different biochemical or physical environments in biological samples has not yet been formally described, because an adequate and general theoretical framework is lacking. Here, we develop a mathematical characterization of the biochemical resolution in fluorescence detection with Fisher information analysis. To improve the precision and the resolution of quantitative imaging methods, we demonstrate strategies for the optimization of fluorescence lifetime, fluorescence anisotropy and hyperspectral detection, as well as different multi-dimensional techniques. We describe optimized imaging protocols, provide optimization algorithms and describe precision and resolving power in biochemical imaging thanks to the analysis of the general properties of Fisher information in fluorescence detection. These strategies enable the optimal use of the information content available within the limited photon-budget typically available in fluorescence microscopy. This theoretical foundation leads to a generalized strategy for the optimization of multi-dimensional optical detection, and demonstrates how the parallel detection of all properties of fluorescence can maximize the biochemical resolving power of fluorescence microscopy, an approach we term Hyper Dimensional Imaging Microscopy (HDIM). Our work provides a theoretical framework for the description of the biochemical resolution in fluorescence microscopy, irrespective of spatial resolution, and for the development of a new class of microscopes that exploit multi-parametric detection systems. PMID:24204821
Geometric approach to the design of an imaging probe to evaluate the iridocorneal angle structures
NASA Astrophysics Data System (ADS)
Hong, Xun Jie Jeesmond; V. K., Shinoj; Murukeshan, V. M.; Baskaran, M.; Aung, Tin
2017-06-01
Photographic imaging methods allow the tracking of anatomical changes in the iridocorneal angle structures and the monitoring of treatment responses overtime. In this work, we aim to design an imaging probe to evaluate the iridocorneal angle structures using geometrical optics. We first perform an analytical analysis on light propagation from the anterior chamber of the eye to the exterior medium using Snell's law. This is followed by adopting a strategy to achieve uniform near field irradiance, by simplifying the complex non-rotational symmetric irradiance distribution of LEDs tilted at an angle. The optimization is based on the geometric design considerations of an angled circular ring array of 4 LEDs (or a 2 × 2 square LED array). The design equation give insights on variable parameters such as the illumination angle of the LEDs, ring array radius, viewing angle of the LEDs, and the working distance. A micro color CCD video camera that has sufficient resolution to resolve the iridocorneal angle structures at the required working distance is then chosen. The proposed design aspects fulfil the safety requirements recommended by the International Commission on Non-ionizing Radiation Protection.
A precise laboratory goniometer system to collect spectral BRDF data of materials
NASA Astrophysics Data System (ADS)
Jiao, Guangping; Jiao, Ziti; Wang, Jie; Zhang, Hu; Dong, Yadong
2014-11-01
This paper presents a precise laboratory goniometer system to quickly collect bidirectional reflectance distribution factor(BRDF)of typical materials such soil, canopy and artificial materials in the laboratory. The system consists of the goniometer, SVC HR1024 spectroradiometer, and xenon long-arc lamp as light source. the innovation of cantilever slab can reduce the shadow of the goniometer in the principle plane. The geometric precision of the footprint centre is better than +/-4cm in most azimuth directions, and the angle-controlling accuracy is better than 0.5°. The light source keeps good stability, with 0.8% irradiance decrease in 3 hours. But the large areal heterogeneity of the light source increase the data processing difficulty to capture the accurate BRDF. First measurements are taken from soil in a resolution of 15° and 30° in zenith and azimuth direction respectively, with the +/-50° biggest view angle. More observations are taken in the hot-spot direction. The system takes about 40 minutes to complete all measurements. A spectralon panel is measured at the beginning and end of the whole period. A simple interactive interface on the computer can automatically control all operations of the goniometer and data-processing. The laboratory experiment of soil layer and grass lawn shows that the goniometer can capture the the multi-angle variation of BRDF.
Non-rigid Earth rotation series
NASA Astrophysics Data System (ADS)
Pashkevich, V. V.
2008-04-01
The last years a lot of attempts to derive a high-precision theory of the non-rigid Earth rotation was carried out. For these purposes the different transfer functions are used. Usually these transfer func- tions are applied to the series representing the nutation in longitude and in obliquity of the rigid Earth rotation with respect to the ecliptic of date. The aim of this investigation is a construction of the new high- precision non-rigid Earth rotation series (SN9000), dynamically adequate to the DE404/LE404 ephemeris over 2000 years, which are expressed as a function of Euler angles ψ, θ and φ with respect to the fixed ecliptic plane and equinox J2000.0. The early stages of the previous investigation: 1. The high-precision numerical solution of the rigid Earth rotation have been constructed (V.V.Pashkevich, G.I.Eroshkin and A.Brzezinski, 2004), (V.V.Pashkevich and G.I.Eroshkin, Proceedings of Journees 2004). The initial con- ditions have been calculated from SMART97 (P.Bretagnon, G.Francou, P.Rocher, J.L.Simon,1998). The discrepancies between the numerical solution and the semi-analytical solution SMART97 were obtained in Euler angles over 2000 years with one-day spacing. 2. Investigation of the discrepancies is carried out by the least squares and by the spectral analysis algorithms (V.V.Pashkevich and G.I.Eroshkin, Proceedings of Journees 2005). The high-precision rigid Earth rotation series S9000 are determined (V.V.Pashkevich and G.I.Eroshkin, 2005 ). The next stage of this investigation: 3. The new high-precision non-rigid Earth rotation series (SN9000), which are expressed as a function of Euler angles, are constructed by using the method (P.Bretagnon, P.M.Mathews, J.-L.Simon: 1999) and the transfer function MHB2002 (Mathews, P. M., Herring, T. A., and Buffett B. A., 2002).
A New Undergraduate Course on the Physics of Space Situational Awareness
2009-09-01
optically resolved imaging, radiometry and photometry , radar detection and tracking, orbital prediction, debris and collision avoidance, detection of...angles only). In the radio receiver lo satellites an site to send get time de satellites cr obtained fr Images take frequency lab cated at USAF d...How it moves and where it is: Astrodynamics 22 Radar Imaging 2 Orbital Dynamics and Types of Orbits 3 Satellite Types 23 Resolved Visible
Detection of intestinal dysplasia using angle-resolved low coherence interferometry
Terry, Neil; Zhu, Yizheng; Thacker, Julie K. M.; Migaly, John; Guy, Cynthia; Mantyh, Christopher R.; Wax, Adam
2011-01-01
Angle-resolved low coherence interferometry (a/LCI) is an optical biopsy technique that allows for depth-resolved, label-free measurement of the average size and optical density of cell nuclei in epithelial tissue to assess the tissue health. a/LCI has previously been used clinically to identify the presence of dysplasia in Barrett's Esophagus patients undergoing routine surveillance. We present the results of a pilot, ex vivo study of tissues from 27 patients undergoing partial colonic resection surgery, conducted to evaluate the ability of a/LCI to identify dysplasia. Performance was determined by comparing the nuclear morphology measurements with pathological assessment of co-located physical biopsies. A statistically significant correlation between increased average nuclear size, reduced nuclear density, and the presence of dysplasia was noted at the basal layer of the epithelium, at a depth of 200 to 300 μm beneath the tissue surface. Using a decision line determined from a receiver operating characteristic, a/LCI was able to separate dysplastic from healthy tissues with a sensitivity of 92.9% (13/14), a specificity of 83.6% (56/67), and an overall accuracy of 85.2% (69/81). The study illustrates the extension of the a/LCI technique to the detection of intestinal dysplasia, and demonstrates the need for future in vivo studies. PMID:22029349
Detection of intestinal dysplasia using angle-resolved low coherence interferometry
NASA Astrophysics Data System (ADS)
Terry, Neil; Zhu, Yizheng; Thacker, Julie K. M.; Migaly, John; Guy, Cynthia; Mantyh, Christopher R.; Wax, Adam
2011-10-01
Angle-resolved low coherence interferometry (a/LCI) is an optical biopsy technique that allows for depth-resolved, label-free measurement of the average size and optical density of cell nuclei in epithelial tissue to assess the tissue health. a/LCI has previously been used clinically to identify the presence of dysplasia in Barrett's Esophagus patients undergoing routine surveillance. We present the results of a pilot, ex vivo study of tissues from 27 patients undergoing partial colonic resection surgery, conducted to evaluate the ability of a/LCI to identify dysplasia. Performance was determined by comparing the nuclear morphology measurements with pathological assessment of co-located physical biopsies. A statistically significant correlation between increased average nuclear size, reduced nuclear density, and the presence of dysplasia was noted at the basal layer of the epithelium, at a depth of 200 to 300 μm beneath the tissue surface. Using a decision line determined from a receiver operating characteristic, a/LCI was able to separate dysplastic from healthy tissues with a sensitivity of 92.9% (13/14), a specificity of 83.6% (56/67), and an overall accuracy of 85.2% (69/81). The study illustrates the extension of the a/LCI technique to the detection of intestinal dysplasia, and demonstrates the need for future in vivo studies.
Precision flux density measurements of the giant planets at 8420 MHz
NASA Technical Reports Server (NTRS)
Turegano, J. A.; Klein, M. J.
1981-01-01
Precision measurements of the 3.56 cm flux densities of Jupiter, Saturn, Uranus, and Neptune are reported. The results are compared with previously published measurements as a means of: remotely sensing long-term changes in the microwave emission from the atmospheres of these planets and measuring the effects of Saturn's rings on the disk temperature as observed from earth at different ring inclination angles.
ERIC Educational Resources Information Center
Hsu, Wei-Tai; Bahrim, Cristian
2009-01-01
Based on our novel method recently published in the "Am. J. Phys." 77 337-43 (2009) for finding precise values of the indices of refraction for dielectrics from measurements of the polarized light reflected by the surface, in this paper we propose an improved technique for finding Brewster angles with a better precision, of 0.001 degrees, using…
NASA Astrophysics Data System (ADS)
Senkovskiy, Boris V.; Usachov, Dmitry Yu; Fedorov, Alexander V.; Haberer, Danny; Ehlen, Niels; Fischer, Felix R.; Grüneis, Alexander
2018-07-01
To understand the optical and transport properties of graphene nanoribbons, an unambiguous determination of their electronic band structure is needed. In this work we demonstrate that the photoemission intensity of each valence sub-band, formed due to the quantum confinement in quasi-one-dimensional (1D) graphene nanoribbons, is a peaked function of the two-dimensional (2D) momentum. We resolve the long-standing discrepancy regarding the valence band effective mass () of armchair graphene nanoribbons with a width of N = 7 carbon atoms (7-AGNRs). In particular, angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling spectroscopy report ≈0.2 and ≈0.4 of the free electron mass (m e ), respectively. ARPES mapping in the full 2D momentum space identifies the experimental conditions for obtaining a large intensity for each of the three highest valence 1D sub-bands. Our detail map reveals that previous ARPES experiments have incorrectly assigned the second sub-band as the frontier one. The correct frontier valence sub-band for 7-AGNRs is only visible in a narrow range of emission angles. For this band we obtain an ARPES derived effective mass of 0.4 m e , a charge carrier velocity in the linear part of the band of 0.63 × 106 m s‑1 and an energy separation of only ≈60 meV to the second sub-band. Our results are of importance not only for the growing research field of graphene nanoribbons but also for the community, which studies quantum confined systems.
Strocov, V. N.; Schmitt, T.; Flechsig, U.; Schmidt, T.; Imhof, A.; Chen, Q.; Raabe, J.; Betemps, R.; Zimoch, D.; Krempasky, J.; Wang, X.; Grioni, M.; Piazzalunga, A.; Patthey, L.
2010-01-01
The concepts and technical realisation of the high-resolution soft X-ray beamline ADRESS operating in the energy range from 300 to 1600 eV and intended for resonant inelastic X-ray scattering (RIXS) and angle-resolved photoelectron spectroscopy (ARPES) are described. The photon source is an undulator of novel fixed-gap design where longitudinal movement of permanent magnetic arrays controls not only the light polarization (including circular and 0–180° rotatable linear polarizations) but also the energy without changing the gap. The beamline optics is based on the well established scheme of plane-grating monochromator operating in collimated light. The ultimate resolving power E/ΔE is above 33000 at 1 keV photon energy. The choice of blazed versus lamellar gratings and optimization of their profile parameters is described. Owing to glancing angles on the mirrors as well as optimized groove densities and profiles of the gratings, the beamline is capable of delivering high photon flux up to 1 × 1013 photons s−1 (0.01% BW)−1 at 1 keV. Ellipsoidal refocusing optics used for the RIXS endstation demagnifies the vertical spot size down to 4 µm, which allows slitless operation and thus maximal transmission of the high-resolution RIXS spectrometer delivering E/ΔE > 11000 at 1 keV photon energy. Apart from the beamline optics, an overview of the control system is given, the diagnostics and software tools are described, and strategies used for the optical alignment are discussed. An introduction to the concepts and instrumental realisation of the ARPES and RIXS endstations is given. PMID:20724785
Spatially Resolved Spectroscopy and Coronagraphic Imaging of the TW Hydrae Circumstellar Disk
NASA Astrophysics Data System (ADS)
Roberge, Aki; Weinberger, Alycia J.; Malumuth, Eliot M.
2005-04-01
We present the first spatially resolved spectrum of scattered light from the TW Hydrae protoplanetary disk. This nearly face-on disk is optically thick, surrounding a classical T Tauri star in the nearby 10 Myr old TW Hya association. The spectrum was taken with the Hubble Space Telescope (HST) STIS CCD, providing resolution R~360 over the wavelength range 5250-10300 Å. Spatially resolved spectroscopy of circumstellar disks is difficult because of the high contrast ratio between the bright star and faint disk. Our novel observations provide optical spectra of scattered light from the disk between 40 and 155 AU from the star. The scattered light has the same color as the star (gray scattering) at all radii except the innermost region. This likely indicates that the scattering dust grains are larger than about 1 μm all the way out to large radii. From the spectroscopic data, we also obtained radial profiles of the integrated disk brightness at two position angles, over almost the same region as previously observed in HST WFPC2 and NICMOS coronagraphic images (35 to 173 AU from the star). The profiles have the same shape as the earlier ones, but show a small azimuthal asymmetry in the disk not previously noted. Our STIS broadband coronagraphic images of TW Hya confirm the reality of this asymmetry, and show that the disk surface brightness inside 140 AU has a sinusoidal dependence on azimuthal angle. The maximum brightness occurs at a position angle of 233.6d+/-5.7d east of north. This might be caused by the combination of forward scattering and an increase in inclination in the inner region of the disk, suggesting that the TW Hya disk has a warp like that seen in the β Pictoris debris disk.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Zwan, B J; University of Newcastle, Newcastle, NSW; Barnes, M
2016-06-15
Purpose: To automate gantry-resolved linear accelerator (linac) quality assurance (QA) for volumetric modulated arc therapy (VMAT) using an electronic portal imaging device (EPID). Methods: A QA system for VMAT was developed that uses an EPID, frame-grabber assembly and in-house developed image processing software. The system relies solely on the analysis of EPID image frames acquired without the presence of a phantom. Images were acquired at 8.41 frames per second using a frame grabber and ancillary acquisition computer. Each image frame was tagged with a gantry angle from the linac’s on-board gantry angle encoder. Arc-dynamic QA plans were designed to assessmore » the performance of each individual linac component during VMAT. By analysing each image frame acquired during the QA deliveries the following eight machine performance characteristics were measured as a function of gantry angle: MLC positional accuracy, MLC speed constancy, MLC acceleration constancy, MLC-gantry synchronisation, beam profile constancy, dose rate constancy, gantry speed constancy, dose-gantry angle synchronisation and mechanical sag. All tests were performed on a Varian iX linear accelerator equipped with a 120 leaf Millennium MLC and an aS1000 EPID (Varian Medical Systems, Palo Alto, CA, USA). Results: Machine performance parameters were measured as a function of gantry angle using EPID imaging and compared to machine log files and the treatment plan. Data acquisition is currently underway at 3 centres, incorporating 7 treatment units, at 2 weekly measurement intervals. Conclusion: The proposed system can be applied for streamlined linac QA and commissioning for VMAT. The set of test plans developed can be used to assess the performance of each individual components of the treatment machine during VMAT deliveries as a function of gantry angle. The methodology does not require the setup of any additional phantom or measurement equipment and the analysis is fully automated to allow for regular routine testing.« less
Cubison, M. J.; Jimenez, J. L.
2015-06-05
Least-squares fitting of overlapping peaks is often needed to separately quantify ions in high-resolution mass spectrometer data. A statistical simulation approach is used to assess the statistical precision of the retrieved peak intensities. The sensitivity of the fitted peak intensities to statistical noise due to ion counting is probed for synthetic data systems consisting of two overlapping ion peaks whose positions are pre-defined and fixed in the fitting procedure. The fitted intensities are sensitive to imperfections in the m/Q calibration. These propagate as a limiting precision in the fitted intensities that may greatly exceed the precision arising from counting statistics.more » The precision on the fitted peak intensity falls into one of three regimes. In the "counting-limited regime" (regime I), above a peak separation χ ~ 2 to 3 half-widths at half-maximum (HWHM), the intensity precision is similar to that due to counting error for an isolated ion. For smaller χ and higher ion counts (~ 1000 and higher), the intensity precision rapidly degrades as the peak separation is reduced ("calibration-limited regime", regime II). Alternatively for χ < 1.6 but lower ion counts (e.g. 10–100) the intensity precision is dominated by the additional ion count noise from the overlapping ion and is not affected by the imprecision in the m/Q calibration ("overlapping-limited regime", regime III). The transition between the counting and m/Q calibration-limited regimes is shown to be weakly dependent on resolving power and data spacing and can thus be approximated by a simple parameterisation based only on peak intensity ratios and separation. A simple equation can be used to find potentially problematic ion pairs when evaluating results from fitted spectra containing many ions. Longer integration times can improve the precision in regimes I and III, but a given ion pair can only be moved out of regime II through increased spectrometer resolving power. As a result, studies presenting data obtained from least-squares fitting procedures applied to mass spectral peaks should explicitly consider these limits on statistical precision.« less
NASA Astrophysics Data System (ADS)
Buckley, Darragh; McCormack, Robert; O'Dwyer, Colm
2017-04-01
The angle-resolved reflectance of high crystalline quality, c-axis oriented ZnO and AZO single and periodic quasi-superlattice (QSL) spin-coated TFT channels materials are presented. The data is analysed using an adapted model to accurately determine the spectral region for optical thickness and corresponding reflectance. The optical thickness agrees very well with measured thickness of 1-20 layered QSL thin films determined by transmission electron microscopy if the reflectance from lowest interference order is used. Directional reflectance for single layers or homogeneous QSLs of ZnO and AZO channel materials exhibit a consistent degree of anti-reflection characteristics from 30 to 60° (~10-12% reflection) for thickness ranging from ~40 nm to 500 nm. The reflectance of AZO single layer thin films is <10% from 30 to 75° at 514.5 nm, and <6% at 632.8 nm from 30-60°. The data show that ZnO and AZO with granular or periodic substructure behave optically as dispersive, continuous thin films of similar thickness, and angle-resolved spectral mapping provides a design rule for transparency or refractive index determination as a function of film thickness, substructure (dispersion) and viewing angle.
NASA Astrophysics Data System (ADS)
Chaban, R.; Pace, D. C.; Marcy, G. R.; Taussig, D.
2016-10-01
Energetic ion losses must be minimized in burning plasmas to maintain fusion power, and existing tokamaks provide access to energetic ion parameter regimes that are relevant to burning machines. A new Fast Ion Loss Detector (FILD) probe on the DIII-D tokamak has been optimized to resolve beam ion losses across a range of 30 - 90 keV in energy and 40° to 80° in pitch angle, thereby providing valuable measurements during many different experiments. The FILD is a magnetic spectrometer; once inserted into the tokamak, the magnetic field allows energetic ions to pass through a collimating aperture and strike a scintillator plate that is imaged by a wide view camera and narrow view photomultiplier tubes (PMTs). The design involves calculating scintillator strike patterns while varying probe geometry. Calculated scintillator patterns are then used to design an optical system that allows adjustment of the focus regions for the 1 MS/s resolved PMTs. A synthetic diagnostic will be used to determine the energy and pitch angle resolution that can be attained in DIII-D experiments. Work supported in part by US DOE under the Science Undergraduate Laboratory Internship (SULI) program and under DE-FC02-04ER54698.
NASA Astrophysics Data System (ADS)
Cuñado, Jose Luis F.; Pedrosa, Javier; Ajejas, Fernando; Perna, Paolo; Miranda, Rodolfo; Camarero, Julio
2017-10-01
Angle- and temperature-dependent vectorial magnetometry measurements are necessary to disentangle the effective magnetic symmetry in magnetic nanostructures. Here we present a detailed study on an Fe(1 0 0) thin film system with competing collinear biaxial (four-fold symmetry) and uniaxial (two-fold) magnetic anisotropies, carried out with our recently developed full angular/broad temperature range/vectorial-resolved magneto-optical Kerr effect magnetometer, named TRISTAN. The data give direct views on the angular and temperature dependence of the magnetization reversal pathways, from which characteristic axes, remanences, critical fields, domain wall types, and effective magnetic symmetry are obtained. In particular, although the remanence shows four-fold angular symmetry for all investigated temperatures (15 K-400 K), the critical fields show strong temperature and angular dependencies and the reversal mechanism changes for specific angles at a given (angle-dependent) critical temperature, showing signatures of an additional collinear two-fold symmetry. This symmetry-breaking is more relevant as temperature increases to room temperature. It originates from the competition between two anisotropy contributions with different symmetry and temperature evolution. The results highlight the importance of combining temperature and angular studies, and the need to look at different magnetic parameters to unravel the underlying magnetic symmetries and temperature evolutions of the symmetry-breaking effects in magnetic nanostructures.
Spin-resolved electron waiting times in a quantum-dot spin valve
NASA Astrophysics Data System (ADS)
Tang, Gaomin; Xu, Fuming; Mi, Shuo; Wang, Jian
2018-04-01
We study the electronic waiting-time distributions (WTDs) in a noninteracting quantum-dot spin valve by varying spin polarization and the noncollinear angle between the magnetizations of the leads using the scattering matrix approach. Since the quantum-dot spin valve involves two channels (spin up and down) in both the incoming and outgoing channels, we study three different kinds of WTDs, which are two-channel WTD, spin-resolved single-channel WTD, and cross-channel WTD. We analyze the behaviors of WTDs in short times, correlated with the current behaviors for different spin polarizations and noncollinear angles. Cross-channel WTD reflects the correlation between two spin channels and can be used to characterize the spin-transfer torque process. We study the influence of the earlier detection on the subsequent detection from the perspective of cross-channel WTD, and define the influence degree quantity as the cumulative absolute difference between cross-channel WTDs and first-passage time distributions to quantitatively characterize the spin-flip process. We observe that influence degree versus spin-transfer torque for different noncollinear angles as well as different polarizations collapse into a single curve showing universal behaviors. This demonstrates that cross-channel WTDs can be a pathway to characterize spin correlation in spintronics system.
NASA Astrophysics Data System (ADS)
Lee, Austin W. H.; Kim, Dongho; Gates, Byron D.
2018-04-01
The thickness of alcohol based monolayers on silicon oxide surfaces were investigated using angle-resolved X-ray photoelectron spectroscopy (ARXPS). Advantages of using alcohols as building blocks for the formation of monolayers include their widespread availability, ease of handling, and stability against side reactions. Recent progress in microwave assisted reactions demonstrated the ease of forming uniform monolayers with alcohol based reagents. The studies shown herein provide a detailed investigation of the thickness of monolayers prepared from a series of aliphatic alcohols of different chain lengths. Monolayers of 1-butanol, 1-hexanol, 1-octanol, 1-decanol, and 1-dodecanol were each successfully formed through microwave assisted reactions and characterized by ARXPS techniques. The thickness of these monolayers consistently increased by ∼1.0 Å for every additional methylene (CH2) within the hydrocarbon chain of the reagents. Tilt angles of the molecules covalently attached to silicon oxide surfaces were estimated to be ∼35° for each type of reagent. These results were consistent with the observations reported for thiol based or silane based monolayers on either gold or silicon oxide surfaces, respectively. The results of this study also suggest that the alcohol based monolayers are uniform at a molecular level.
The Physics of Ultracold Sr2 Molecules: Optical Production and Precision Measurement
2013-01-01
causing stimulated emission. The wavelength of the feedback light is determined by the angle of the feedback mirror . The zeroth order is the output from...with representative mirror , diffraction grating and diode housing (right). . . . . . . . . . . . . . . . . . . . . . . . . . . . . 22 2.14 Schematic of...of the feedback light is determined by the angle of the feedback mirror . The zeroth order is the output from the ECDL. . . . . . . . . . . . 23 2.15
Investigation of an optical sensor for small tilt angle detection of a precision linear stage
NASA Astrophysics Data System (ADS)
Saito, Yusuke; Arai, Yoshikazu; Gao, Wei
2010-05-01
This paper presents evaluation results of the characteristics of the angle sensor based on the laser autocollimation method for small tilt angle detection of a precision linear stage. The sensor consists of a laser diode (LD) as the light source, and a quadrant photodiode (QPD) as the position-sensing detector. A small plane mirror is mounted on the moving table of the stage as a target mirror for the sensor. This optical system has advantages of high sensitivity, fast response speed and the ability for two-axis angle detection. On the other hand, the sensitivity of the sensor is determined by the size of the optical spot focused on the QPD, which is a function of the diameter of the laser beam projected onto the target mirror. Because the diameter is influenced by the divergence of the laser beam, this paper focuses on the relationship between the sensor sensitivity and the moving position of the target mirror (sensor working distance) over the moving stroke of the stage. The main error components that influence the sensor sensitivity are discussed and the optimal conditions of the optical system of the sensor are analyzed. The experimental result about evaluation of the effective working distance is also presented.
Okamoto, Shigetoshi; Mizu-uchi, Hideki; Okazaki, Ken; Hamai, Satoshi; Tashiro, Yasutaka; Nakahara, Hiroyuki; Iwamoto, Yukihide
2016-01-01
The first purpose of this study was to compare the reproducibility of two-dimensional (2D) and three-dimensional (3D) measurements for preoperative planning of the femoral side in total knee arthroplasty (TKA). The second purpose was to evaluate the factors affecting the differences between the 2D and 3D measurements. Two-dimensional and 3D measurements for preoperative planning of the femoral side in TKA were evaluated in 75 varus knees with osteoarthritis. The femoral valgus angle, defined as the angle between the mechanical and anatomical axes of the femur, and the clinical rotation angle and surgical rotation angle, defined by the angles between the posterior condylar line and the clinical or surgical transepicondylar axes, respectively, were analysed using 2D (radiographs and axial CT slices) and 3D (3D bone models reconstructed from CT images) measurements. For all variables, 3D measurements were more reliable and reproducible than 2D measurements. The medians and ranges of the clinical rotation angle and surgical rotation angle were 6.6° (-1.7° to 12.1°) and 2.3° (-2.5° to 8.6°) in 2D, and 7.1° (2.7° to 11.4°) and 3.0° (-2.0° to 7.5°) in 3D. Varus/valgus alteration of the CT scanning direction relative to the mechanical axis affected the difference in clinical rotation angles between 2D and 3D measurements. Significantly, smaller values of the clinical rotation angle and surgical rotation angle were obtained by 2D compared to 3D measurements, which could result in internal rotation of the femoral component even if the surgeon performs the bone cutting precisely. Regarding clinical relevance, first, this study confirmed the reliability of 3D measurements. Second, it underscored the risk of internal rotation of the femoral component when using 2D measurement, even with precise bone cutting technique. These results will help surgeons avoid malpositioning of the femoral component if 2D measurements are used for preoperative planning in TKA. Prospective comparative study, Level Ш.
Stereo-photography of streamers in air
DOE Office of Scientific and Technical Information (OSTI.GOV)
Nijdam, S.; Moerman, J. S.; Briels, T. M. P.
2008-03-10
Standard photographs of streamer discharges show a two-dimensional projection. Here, we present stereophotographic images that resolve their three-dimensional structure. We describe the stereoscopic setup and evaluation, and we present results for positive streamer discharges in air at 0.2-1 bar in a point-plane geometry with a gap distance of 14 cm and a voltage pulse of 47 kV. In this case, an approximately Gaussian distribution of branching angles of 43 deg. {+-}12 deg. is found; these angles do not significantly depend on the distance from the needle or on the gas pressure.
Multiple scattering calculations of relativistic electron energy loss spectra
NASA Astrophysics Data System (ADS)
Jorissen, K.; Rehr, J. J.; Verbeeck, J.
2010-04-01
A generalization of the real-space Green’s-function approach is presented for ab initio calculations of relativistic electron energy loss spectra (EELS) which are particularly important in anisotropic materials. The approach incorporates relativistic effects in terms of the transition tensor within the dipole-selection rule. In particular, the method accounts for relativistic corrections to the magic angle in orientation resolved EELS experiments. The approach is validated by a study of the graphite CK edge, for which we present an accurate magic angle measurement consistent with the predicted value.
NASA Astrophysics Data System (ADS)
Caruso, Fabio; Verdi, Carla; Poncé, Samuel; Giustino, Feliciano
2018-04-01
We develop a first-principles approach based on many-body perturbation theory to investigate the effects of the interaction between electrons and carrier plasmons on the electronic properties of highly doped semiconductors and oxides. Through the evaluation of the electron self-energy, we account simultaneously for electron-plasmon and electron-phonon coupling in theoretical calculations of angle-resolved photoemission spectra, electron linewidths, and relaxation times. We apply this methodology to electron-doped anatase TiO2 as an illustrative example. The simulated spectra indicate that electron-plasmon coupling in TiO2 underpins the formation of satellites at energies comparable to those of polaronic spectral features. At variance with phonons, however, the energy of plasmons and their spectral fingerprints depends strongly on the carrier concentration, revealing a complex interplay between plasmon and phonon satellites. The electron-plasmon interaction accounts for approximately 40% of the total electron-boson interaction strength, and it is key to improve the agreement with measured quasiparticle spectra.
Spatiotemporal Evolution of Runaway Electron Momentum Distributions in Tokamaks
Paz-Soldan, Carlos; Cooper, Christopher M.; Aleynikov, Pavel; ...
2017-06-22
Novel spatial, temporal, and energetically resolved measurements of bremsstrahlung hard-x-ray (HXR) emission from runaway electron (RE) populations in tokamaks reveal nonmonotonic RE distribution functions whose properties depend on the interplay of electric field acceleration with collisional and synchrotron damping. Measurements are consistent with theoretical predictions of momentum-space attractors that accumulate runaway electrons. RE distribution functions are measured to shift to a higher energy when the synchrotron force is reduced by decreasing the toroidal magnetic field strength. Increasing the collisional damping by increasing the electron density (at a fixed magnetic and electric field) reduces the energy of the nonmonotonic feature andmore » reduces the HXR growth rate at all energies. Higher-energy HXR growth rates extrapolate to zero at the expected threshold electric field for RE sustainment, while low-energy REs are anomalously lost. The compilation ofHXR emission from different sight lines into the plasma yields energy and pitch-angle-resolved RE distributions and demonstrates increasing pitch-angle and radial gradients with energy.« less
Jobst, Johannes; van der Torren, Alexander J. H.; Krasovskii, Eugene E.; Balgley, Jesse; Dean, Cory R.; Tromp, Rudolf M.; van der Molen, Sense Jan
2016-01-01
High electron mobility is one of graphene's key properties, exploited for applications and fundamental research alike. Highest mobility values are found in heterostructures of graphene and hexagonal boron nitride, which consequently are widely used. However, surprisingly little is known about the interaction between the electronic states of these layered systems. Rather pragmatically, it is assumed that these do not couple significantly. Here we study the unoccupied band structure of graphite, boron nitride and their heterostructures using angle-resolved reflected-electron spectroscopy. We demonstrate that graphene and boron nitride bands do not interact over a wide energy range, despite their very similar dispersions. The method we use can be generally applied to study interactions in van der Waals systems, that is, artificial stacks of layered materials. With this we can quantitatively understand the ‘chemistry of layers' by which novel materials are created via electronic coupling between the layers they are composed of. PMID:27897180
Avila, José; Razado, Ivy; Lorcy, Stéphane; Fleurier, Romain; Pichonat, Emmanuelle; Vignaud, Dominique; Wallart, Xavier; Asensio, María C.
2013-01-01
The ability to produce large, continuous and defect free films of graphene is presently a major challenge for multiple applications. Even though the scalability of graphene films is closely associated to a manifest polycrystalline character, only a few numbers of experiments have explored so far the electronic structure down to single graphene grains. Here we report a high resolution angle and lateral resolved photoelectron spectroscopy (nano-ARPES) study of one-atom thick graphene films on thin copper foils synthesized by chemical vapor deposition. Our results show the robustness of the Dirac relativistic-like electronic spectrum as a function of the size, shape and orientation of the single-crystal pristine grains in the graphene films investigated. Moreover, by mapping grain by grain the electronic dynamics of this unique Dirac system, we show that the single-grain gap-size is 80% smaller than the multi-grain gap recently reported by classical ARPES. PMID:23942471
NASA Astrophysics Data System (ADS)
Ito, S.; Feng, B.; Arita, M.; Someya, T.; Chen, W.-C.; Takayama, A.; Iimori, T.; Namatame, H.; Taniguchi, M.; Cheng, C.-M.; Tang, S.-J.; Komori, F.; Matsuda, I.
2018-04-01
Alkali-metal adsorption on the surface of materials is widely used for in situ surface electron doping, particularly for observing unoccupied band structures by angle-resolved photoemission spectroscopy (ARPES). However, the effects of alkali-metal atoms on the resulting band structures have yet to be fully investigated, owing to difficulties in both experiments and calculations. Here, we combine ARPES measurements on cesium-adsorbed ultrathin bismuth films with first-principles calculations of the electronic charge densities and demonstrate a simple method to evaluate alkali-metal induced band deformation. We reveal that deformation of bismuth surface bands is directly correlated with vertical charge-density profiles at each electronic state of bismuth. In contrast, a change in the quantized bulk bands is well described by a conventional rigid-band-shift picture. We discuss these two aspects of the band deformation holistically, considering spatial distributions of the electronic states and cesium-bismuth hybridization, and provide a prescription for applying alkali-metal adsorption to a wide range of materials.
NASA Astrophysics Data System (ADS)
Heiler, M.; Chassé, A.; Schindler, K.-M.; Hollering, M.; Neddermeyer, H.
2000-05-01
We have prepared ordered thin films of CoO by evaporating cobalt in an O 2 atmosphere on to a heated (500 K) Ag(100) substrate. The geometric and electronic structure of the films was characterized by means of Auger electron diffraction (AED) and angle-resolved photoemission spectroscopy (ARUPS), respectively. The experimental AED results were compared with simulated data, which showed that the film grows in (100) orientation on the Ag(100) substrate. Synchrotron-radiation-induced photoemission investigations were performed in the photon energy range from 25 eV to 67 eV. The dispersion of the transitions was found to be similar to that of previous results on a single-crystal CoO(100) surface. The resonance behaviour of the photoemission lines in the valence-band region was investigated by constant-initial-state (CIS) spectroscopy. The implications of this behaviour for assignment of the photoemission lines to specific electronic transitions is discussed and compared with published theoretical models of the electronic structure.
SmB6 electron-phonon coupling constant from time- and angle-resolved photoelectron spectroscopy
NASA Astrophysics Data System (ADS)
Sterzi, A.; Crepaldi, A.; Cilento, F.; Manzoni, G.; Frantzeskakis, E.; Zacchigna, M.; van Heumen, E.; Huang, Y. K.; Golden, M. S.; Parmigiani, F.
2016-08-01
SmB6 is a mixed valence Kondo system resulting from the hybridization between localized f electrons and delocalized d electrons. We have investigated its out-of-equilibrium electron dynamics by means of time- and angle-resolved photoelectron spectroscopy. The transient electronic population above the Fermi level can be described by a time-dependent Fermi-Dirac distribution. By solving a two-temperature model that well reproduces the relaxation dynamics of the effective electronic temperature, we estimate the electron-phonon coupling constant λ to range from 0.13 ±0.03 to 0.04 ±0.01 . These extremes are obtained assuming a coupling of the electrons with either a phonon mode at 10 or 19 meV. A realistic value of the average phonon energy will give an actual value of λ within this range. Our results provide an experimental report on the material electron-phonon coupling, contributing to both the electronic transport and the macroscopic thermodynamic properties of SmB6.
Jin, Wencan; Yeh, Po-Chun; Zaki, Nader; Zhang, Datong; Sadowski, Jerzy T; Al-Mahboob, Abdullah; van der Zande, Arend M; Chenet, Daniel A; Dadap, Jerry I; Herman, Irving P; Sutter, Peter; Hone, James; Osgood, Richard M
2013-09-06
We report on the evolution of the thickness-dependent electronic band structure of the two-dimensional layered-dichalcogenide molybdenum disulfide (MoS2). Micrometer-scale angle-resolved photoemission spectroscopy of mechanically exfoliated and chemical-vapor-deposition-grown crystals provides direct evidence for the shifting of the valence band maximum from Γ to K, for the case of MoS2 having more than one layer, to the case of single-layer MoS2, as predicted by density functional theory. This evolution of the electronic structure from bulk to few-layer to monolayer MoS2 had earlier been predicted to arise from quantum confinement. Furthermore, one of the consequences of this progression in the electronic structure is the dramatic increase in the hole effective mass, in going from bulk to monolayer MoS2 at its Brillouin zone center, which is known as the cause for the decreased carrier mobility of the monolayer form compared to that of bulk MoS2.
NASA Astrophysics Data System (ADS)
Rienks, E. D. L.; ńrrälä, M.; Lindroos, M.; Roth, F.; Tabis, W.; Yu, G.; Greven, M.; Fink, J.
2014-09-01
We use polarization-dependent angle-resolved photoemission spectroscopy (ARPES) to study the high-energy anomaly (HEA) in the dispersion of Nd2-xCexCuO4, x =0.123. We find that at particular photon energies the anomalous, waterfall-like dispersion gives way to a broad, continuous band. This suggests that the HEA is a matrix element effect: it arises due to a suppression of the intensity of the broadened quasiparticle band in a narrow momentum range. We confirm this interpretation experimentally, by showing that the HEA appears when the matrix element is suppressed deliberately by changing the light polarization. Calculations of the matrix element using atomic wave functions and simulation of the ARPES intensity with one-step model calculations provide further evidence for this scenario. The possibility to detect the full quasiparticle dispersion further allows us to extract the high-energy self-energy function near the center and at the edge of the Brillouin zone.
Rienks, E D L; Ärrälä, M; Lindroos, M; Roth, F; Tabis, W; Yu, G; Greven, M; Fink, J
2014-09-26
We use polarization-dependent angle-resolved photoemission spectroscopy (ARPES) to study the high-energy anomaly (HEA) in the dispersion of Nd(2-x)Ce(x)CuO₄, x=0.123. We find that at particular photon energies the anomalous, waterfall-like dispersion gives way to a broad, continuous band. This suggests that the HEA is a matrix element effect: it arises due to a suppression of the intensity of the broadened quasiparticle band in a narrow momentum range. We confirm this interpretation experimentally, by showing that the HEA appears when the matrix element is suppressed deliberately by changing the light polarization. Calculations of the matrix element using atomic wave functions and simulation of the ARPES intensity with one-step model calculations provide further evidence for this scenario. The possibility to detect the full quasiparticle dispersion further allows us to extract the high-energy self-energy function near the center and at the edge of the Brillouin zone.
ARPES study of the epitaxially grown topological crystalline insulator SnTe(111)
Zhang, Yi; Liu, Zhongkai; Zhou, Bo; ...
2016-10-18
We present that SnTe is a prototypical topological crystalline insulator, in which the gapless surface state is protected by a crystal symmetry. The hallmark of the topological properties in SnTe is the Dirac cones projected to the surfaces with mirror symmetry, stemming from the band inversion near the L points of its bulk Brillouin zone, which can be measured by angle-resolved photoemission. We have obtained the (111) surface of SnTe film by molecular beam epitaxy on BaF 2(111) substrate. Photon-energy-dependence of in situ angle-resolved photoemission, covering multiple Brillouin zones in the direction perpendicular to the (111) surface, demonstrate the projected Dirac cones at themore » $$\\overline{Γ}$$ and $$\\overline{M}$$ points of the surface Brillouin zone. Additionally, we observe a Dirac-cone-like band structure at the Γ point of the bulk Brillouin zone, whose Dirac energy is largely different from those at the $$\\overline{Γ}$$ and $$\\overline{M}$$ points.« less
Anisotropic Electron-Photon and Electron-Phonon Interactions in Black Phosphorus
Ling, Xi; Huang, Shengxi; Hasdeo, Eddwi; ...
2016-03-10
Orthorhombic black phosphorus (BP) and other layered materials, such as gallium telluride (GaTe) and tin selenide (SnSe), stand out among two-dimensional (2D) materials owing to their anisotropic in-plane structure. This anisotropy adds a new dimension to the properties of 2D materials and stimulates the development of angle-resolved photonics and electronics. However, understanding the effect of anisotropy has remained unsatisfactory to-date, as shown by a number of inconsistencies in the recent literatures. We use angle-resolved absorption and Raman spectroscopies to investigate the role of anisotropy on the electron-photon and electron-phonon interactions in BP. We highlight a non-trivial dependence between anisotropies andmore » flake thickness, photon and phonon energies. We show that once understood, the anisotropic optical absorption appears to be a reliable and simple way to identify the crystalline orientation of BP, which cannot be determined from Raman spectroscopy without the explicit consideration of excitation wavelength and flake thickness, as commonly used previously.« less
Time-resolved second-harmonic generation from gold nanoparticle arrays
NASA Astrophysics Data System (ADS)
Ferrara, D. W.; Tetz, K. A.; McMahon, M. D.; Haglund, R. F., Jr.
2007-09-01
We have studied the effects of planar inversion symmetry and particle-coupling of gold nanoparticle (NP) arrays by angle dependent second-harmonic generation (SHG). Time- and angle- resolved measurements were made using a mode-locked Ti:sapphire 800 nm laser onto gold NP arrays with plasmon resonance tuned to match the laser wavelength in order to produce maximum SHG signal. Finite-difference time domain simulations are used to model the near-field distributions for the various geometries and compared to experiment. The arrays were fabricated by focused ion-beam lithography and metal vapor deposition followed by standard lift-off protocols, producing NPs approximately 20nm high with various in-plane dimensions and interparticle gaps. Above a threshold fluence of ~ 7.3 × 10 -5 mJ/cm2 we find that the SHG scales with the third power of intensity, rather than the second, and atomic-force microscopy shows that the NPs have undergone a reshaping process leading to more nearly spherical shapes.
Matt, C. E.; Fatuzzo, C. G.; Sassa, Y.; ...
2015-10-27
We report an angle-resolved photoemission study of the charge stripe ordered La 1.6–xNd 0.4Sr xCuO 4 (Nd-LSCO) system. A comparative and quantitative line-shape analysis is presented as the system evolves from the overdoped regime into the charge ordered phase. On the overdoped side (x = 0.20), a normal-state antinodal spectral gap opens upon cooling below 80 K. In this process, spectral weight is preserved but redistributed to larger energies. A correlation between this spectral gap and electron scattering is found. A different line shape is observed in the antinodal region of charge ordered Nd-LSCO x = 1/8. Significant low-energy spectralmore » weight appears to be lost. As a result, these observations are discussed in terms of spectral-weight redistribution and gapping originating from charge stripe ordering.« less
NASA Astrophysics Data System (ADS)
Crepaldi, A.; Autès, G.; Gatti, G.; Roth, S.; Sterzi, A.; Manzoni, G.; Zacchigna, M.; Cacho, C.; Chapman, R. T.; Springate, E.; Seddon, E. A.; Bugnon, Ph.; Magrez, A.; Berger, H.; Vobornik, I.; Kalläne, M.; Quer, A.; Rossnagel, K.; Parmigiani, F.; Yazyev, O. V.; Grioni, M.
2017-12-01
MoTe2 has recently been shown to realize in its low-temperature phase the type-II Weyl semimetal (WSM). We investigated by time- and angle- resolved photoelectron spectroscopy (tr-ARPES) the possible influence of the Weyl points on the electron dynamics above the Fermi level EF, by comparing the ultrafast response of MoTe2 in the trivial and topological phases. In the low-temperature WSM phase, we report an enhanced relaxation rate of electrons optically excited to the conduction band, which we interpret as a fingerprint of the local gap closure when Weyl points form. By contrast, we find that the electron dynamics of the related compound WTe2 is slower and temperature independent, consistent with a topologically trivial nature of this material. Our results shows that tr-ARPES is sensitive to the small modifications of the unoccupied band structure accompanying the structural and topological phase transition of MoTe2.
NASA Astrophysics Data System (ADS)
Da Pieve, F.
2016-01-01
A method for mapping the local spin and orbital nature of the ground state of a system via corresponding flip excitations is proposed based on angle-resolved resonant photoemission and related diffraction patterns, obtained here via an ab initio modified one-step theory of photoemission. The analysis is done on the paradigmatic weak itinerant ferromagnet bcc Fe, whose magnetism, a correlation phenomenon given by the coexistence of localized moments and itinerant electrons, and the observed non-Fermi-Liquid behavior at extreme conditions both remain unclear. The combined analysis of energy spectra and diffraction patterns offers a mapping of local pure spin-flip, entangled spin-flip-orbital-flip excitations and chiral transitions with vortexlike wave fronts of photoelectrons, depending on the valence orbital symmetry and the direction of the local magnetic moment. Such effects, mediated by the hole polarization, make resonant photoemission a promising tool to perform a full tomography of the local magnetic properties even in itinerant ferromagnets or macroscopically nonmagnetic systems.
Oda, Toshiro; Aihara, Tomoki; Wakabayashi, Katsuzo
2016-01-01
Nucleators generating new F-actin filaments play important roles in cell activities. Detailed information concerning the events involved in nucleation of actin alone in vitro is fundamental to understanding these processes, but such information has been hard to come by. We addressed the early process of salt-induced polymerization of actin using the time-resolved synchrotron small-angle X-ray scattering (SAXS). Actin molecules in low salt solution maintain a monomeric state by an electrostatic repulsive force between molecules. On mixing with salts, the repulsive force was rapidly screened, causing an immediate formation of many of non-polymerizable dimers. SAXS kinetic analysis revealed that tetramerization gives the highest energetic barrier to further polymerization, and the major nucleation is the formation of helical tetramers. Filaments start to grow rapidly with the formation of pentamers. These findings suggest an acceleration mechanism of actin assembly by a variety of nucleators in cells. PMID:27775032
Lee, Yoojin; Callaghan, Martina F; Nagy, Zoltan
2017-01-01
In magnetic resonance imaging, precise measurements of longitudinal relaxation time ( T 1 ) is crucial to acquire useful information that is applicable to numerous clinical and neuroscience applications. In this work, we investigated the precision of T 1 relaxation time as measured using the variable flip angle method with emphasis on the noise propagated from radiofrequency transmit field ([Formula: see text]) measurements. The analytical solution for T 1 precision was derived by standard error propagation methods incorporating the noise from the three input sources: two spoiled gradient echo (SPGR) images and a [Formula: see text] map. Repeated in vivo experiments were performed to estimate the total variance in T 1 maps and we compared these experimentally obtained values with the theoretical predictions to validate the established theoretical framework. Both the analytical and experimental results showed that variance in the [Formula: see text] map propagated comparable noise levels into the T 1 maps as either of the two SPGR images. Improving precision of the [Formula: see text] measurements significantly reduced the variance in the estimated T 1 map. The variance estimated from the repeatedly measured in vivo T 1 maps agreed well with the theoretically-calculated variance in T 1 estimates, thus validating the analytical framework for realistic in vivo experiments. We concluded that for T 1 mapping experiments, the error propagated from the [Formula: see text] map must be considered. Optimizing the SPGR signals while neglecting to improve the precision of the [Formula: see text] map may result in grossly overestimating the precision of the estimated T 1 values.
Non-contact angle measurement based on parallel multiplex laser feedback interferometry
NASA Astrophysics Data System (ADS)
Zhang, Song; Tan, Yi-Dong; Zhang, Shu-Lian
2014-11-01
We present a novel precise angle measurement scheme based on parallel multiplex laser feedback interferometry (PLFI), which outputs two parallel laser beams and thus their displacement difference reflects the angle variation of the target. Due to its ultrahigh sensitivity to the feedback light, PLFI realizes the direct non-contact measurement of non-cooperative targets. Experimental results show that PLFI has an accuracy of 8″ within a range of 1400″. The yaw of a guide is also measured and the experimental results agree with those of the dual-frequency laser interferometer Agilent 5529A.
Reducing Bolt Preload Variation with Angle-of-Twist Bolt Loading
NASA Technical Reports Server (NTRS)
Thompson, Bryce; Nayate, Pramod; Smith, Doug; McCool, Alex (Technical Monitor)
2001-01-01
Critical high-pressure sealing joints on the Space Shuttle reusable solid rocket motor require precise control of bolt preload to ensure proper joint function. As the reusable solid rocket motor experiences rapid internal pressurization, correct bolt preloads maintain the sealing capability and structural integrity of the hardware. The angle-of-twist process provides the right combination of preload accuracy, reliability, process control, and assembly-friendly design. It improves significantly over previous methods. The sophisticated angle-of-twist process controls have yielded answers to all discrepancies encountered while the simplicity of the root process has assured joint preload reliability.
Grism and immersion grating for space telescope
NASA Astrophysics Data System (ADS)
Ebizuka, Noboru; Oka, Kiko; Yamada, Akiko; Ishikawa, Mami; Kashiwagi, Masako; Kodate, Kashiko; Hirahara, Yasuhiro; Sato, Shuji; Kawabata, Koji S.; Wakaki, Moriaki; Morita, Shin-ya; Simizu, Tomoyuki; Yin, Shaohui; Omori, Hitoshi; Iye, Masanori
2017-11-01
The grism is a versatile dispersion element for an astronomical instrument ranging from ultraviolet to infrared. Major benefit of using a grism in a space application, instead of a reflection grating, is the size reduction of optical system because collimator and following optical elements could locate near by the grism. The surface relief (SR) grism is consisted a transmission grating and a prism, vertex angle of which is adjusted to redirect the diffracted beam straight along the direct vision direction at a specific order and wavelength. The volume phase holographic (VPH) grism consists a thick VPH grating sandwiched between two prisms, as specific order and wavelength is aligned the direct vision direction. The VPH grating inheres ideal diffraction efficiency on a higher dispersion application. On the other hand, the SR grating could achieve high diffraction efficiency on a lower dispersion application. Five grisms among eleven for the Faint Object Camera And Spectrograph (FOCAS) of the 8.2m Subaru Telescope with the resolving power from 250 to 3,000 are SR grisms fabricated by a replication method. Six additional grisms of FOCAS with the resolving power from 3,000 to 7,000 are VPH grisms. We propose "Quasi-Bragg grism" for a high dispersion spectroscopy with wide wavelength range. The germanium immersion grating for instance could reduce 1/64 as the total volume of a spectrograph with a conventional reflection grating since refractive index of germanium is over 4.0 from 1.6 to 20 μm. The prototype immersion gratings for the mid-InfraRed High dispersion Spectrograph (IRHS) are successfully fabricated by a nano-precision machine and grinding cup of cast iron with electrolytic dressing method.
NASA Astrophysics Data System (ADS)
Séférian, Roland; Baek, Sunghye; Boucher, Olivier; Dufresne, Jean-Louis; Decharme, Bertrand; Saint-Martin, David; Roehrig, Romain
2018-01-01
Ocean surface represents roughly 70 % of the Earth's surface, playing a large role in the partitioning of the energy flow within the climate system. The ocean surface albedo (OSA) is an important parameter in this partitioning because it governs the amount of energy penetrating into the ocean or reflected towards space. The old OSA schemes in the ARPEGE-Climat and LMDZ models only resolve the latitudinal dependence in an ad hoc way without an accurate representation of the solar zenith angle dependence. Here, we propose a new interactive OSA scheme suited for Earth system models, which enables coupling between Earth system model components like surface ocean waves and marine biogeochemistry. This scheme resolves spectrally the various contributions of the surface for direct and diffuse solar radiation. The implementation of this scheme in two Earth system models leads to substantial improvements in simulated OSA. At the local scale, models using the interactive OSA scheme better replicate the day-to-day distribution of OSA derived from ground-based observations in contrast to old schemes. At global scale, the improved representation of OSA for diffuse radiation reduces model biases by up to 80 % over the tropical oceans, reducing annual-mean model-data error in surface upwelling shortwave radiation by up to 7 W m-2 over this domain. The spatial correlation coefficient between modeled and observed OSA at monthly resolution has been increased from 0.1 to 0.8. Despite its complexity, this interactive OSA scheme is computationally efficient for enabling precise OSA calculation without penalizing the elapsed model time.
Vision-based in-line fabric defect detection using yarn-specific shape features
NASA Astrophysics Data System (ADS)
Schneider, Dorian; Aach, Til
2012-01-01
We develop a methodology for automatic in-line flaw detection in industrial woven fabrics. Where state of the art detection algorithms apply texture analysis methods to operate on low-resolved ({200 ppi) image data, we describe here a process flow to segment single yarns in high-resolved ({1000 ppi) textile images. Four yarn shape features are extracted, allowing a precise detection and measurement of defects. The degree of precision reached allows a classification of detected defects according to their nature, providing an innovation in the field of automatic fabric flaw detection. The design has been carried out to meet real time requirements and face adverse conditions caused by loom vibrations and dirt. The entire process flow is discussed followed by an evaluation using a database with real-life industrial fabric images. This work pertains to the construction of an on-loom defect detection system to be used in manufacturing practice.
Spatially resolved photodiode response for simulating precise interferometers.
Fernández Barranco, Germán; Tröbs, Michael; Müller, Vitali; Gerberding, Oliver; Seifert, Frank; Heinzel, Gerhard
2016-08-20
Quadrant photodiodes (QPDs) are used in laser interferometry systems to simultaneously detect longitudinal displacement of test masses and angular misalignment between the two interfering beams. The latter is achieved by means of the differential wavefront sensing (DWS) technique, which provides ultra-high precision for measuring angular displacements. We have developed a setup to obtain the spatially resolved response of QPDs that, together with an extension of the simulation software IfoCAD, allows us to use the measured response in simulations and accurately predict the desired longitudinal and DWS phase observables. Three different commercial off-the-shelf QPD candidates for space-based interferometry were characterized. The measured response of one QPD was used in optical simulations. Nonuniformities in the response of the device and crosstalk between segments do not introduce significant variations in the longitudinal and DWS measurands with respect to the standard case when a uniform QPD without crosstalk is used.
Comparative Study on a Solving Model and Algorithm for a Flush Air Data Sensing System
Liu, Yanbin; Xiao, Dibo; Lu, Yuping
2014-01-01
With the development of high-performance aircraft, precise air data are necessary to complete challenging tasks such as flight maneuvering with large angles of attack and high speed. As a result, the flush air data sensing system (FADS) was developed to satisfy the stricter control demands. In this paper, comparative stuides on the solving model and algorithm for FADS are conducted. First, the basic principles of FADS are given to elucidate the nonlinear relations between the inputs and the outputs. Then, several different solving models and algorithms of FADS are provided to compute the air data, including the angle of attck, sideslip angle, dynamic pressure and static pressure. Afterwards, the evaluation criteria of the resulting models and algorithms are discussed to satisfy the real design demands. Futhermore, a simulation using these algorithms is performed to identify the properites of the distinct models and algorithms such as the measuring precision and real-time features. The advantages of these models and algorithms corresponding to the different flight conditions are also analyzed, furthermore, some suggestions on their engineering applications are proposed to help future research. PMID:24859025
Comparative study on a solving model and algorithm for a flush air data sensing system.
Liu, Yanbin; Xiao, Dibo; Lu, Yuping
2014-05-23
With the development of high-performance aircraft, precise air data are necessary to complete challenging tasks such as flight maneuvering with large angles of attack and high speed. As a result, the flush air data sensing system (FADS) was developed to satisfy the stricter control demands. In this paper, comparative stuides on the solving model and algorithm for FADS are conducted. First, the basic principles of FADS are given to elucidate the nonlinear relations between the inputs and the outputs. Then, several different solving models and algorithms of FADS are provided to compute the air data, including the angle of attck, sideslip angle, dynamic pressure and static pressure. Afterwards, the evaluation criteria of the resulting models and algorithms are discussed to satisfy the real design demands. Futhermore, a simulation using these algorithms is performed to identify the properites of the distinct models and algorithms such as the measuring precision and real-time features. The advantages of these models and algorithms corresponding to the different flight conditions are also analyzed, furthermore, some suggestions on their engineering applications are proposed to help future research.
Structural design of morphing trailing edge actuated by SMA
NASA Astrophysics Data System (ADS)
Wang, Qi; Xu, Zhiwei; Zhu, Qian
2013-09-01
In this paper, the morphing trailing edge is designed to achieve the up and down deflection under the aerodynamic load. After a detailed and accurate computational analysis to determine the SMA specifications and layout programs, a solid model is created in CATIA and the structures of the morphing wing trailing edge are produced by CNC machining. A set of DSP measurement and control system is designed to accomplish the controlling experiment of the morphing wing trailing edge. At last, via the force analysis, the trailing edge is fabricated with four sections of aluminum alloy, and the arrangement scheme of SMA wires is determined. Experiment of precise control integral has been performed to survey the control effect. The experiment consists of deflection angle tests of the third joint and the integral structure. Primarily, the ultimate deflection angle is tested in these two experiments. Therefore, the controlling experiment of different angles could be performed within this range. The results show that the deflection error is less than 4%and response time is less than 6.7 s, the precise controlling of the morphing trailing edge is preliminary realized.
Techniques for deriving tissue structure from multiple projection dual-energy x-ray absorptiometry
NASA Technical Reports Server (NTRS)
Feldmesser, Howard S. (Inventor); Charles, Jr., Harry K. (Inventor); Beck, Thomas J. (Inventor); Magee, Thomas C. (Inventor)
2004-01-01
Techniques for deriving bone properties from images generated by a dual-energy x-ray absorptiometry apparatus include receiving first image data having pixels indicating bone mineral density projected at a first angle of a plurality of projection angles. Second image data and third image data are also received. The second image data indicates bone mineral density projected at a different second angle. The third image data indicates bone mineral density projected at a third angle. The third angle is different from the first angle and the second angle. Principal moments of inertia for a bone in the subject are computed based on the first image data, the second image data and the third image data. The techniques allow high-precision, high-resolution dual-energy x-ray attenuation images to be used for computing principal moments of inertia and strength moduli of individual bones, plus risk of injury and changes in risk of injury to a patient.
The Pluto System At Small Phase Angles
NASA Astrophysics Data System (ADS)
Verbiscer, Anne J.; Buie, Marc W.; Binzel, Richard; Ennico, Kimberly; Grundy, William M.; Olkin, Catherine B.; Showalter, Mark Robert; Spencer, John R.; Stern, S. Alan; Weaver, Harold A.; Young, Leslie; New Horizons Science Team
2016-10-01
Hubble Space Telescope observations of the Pluto system acquired during the New Horizons encounter epoch (HST Program 13667, M. Buie, PI) span the phase angle range from 0.06 to 1.7 degrees, enabling the measurement and characterization of the opposition effect for Pluto and its satellites at 0.58 microns using HST WFC3/UVIS with the F350LP filter, which has a broadband response and a pivot wavelength of 0.58 microns. At these small phase angles, differences in the opposition effect width and amplitude appear. The small satellites Nix and Hydra both exhibit a very narrow opposition surge, while the considerably larger moon Charon has a broader opposition surge. Microtextural surface properties derived from the shape and magnitude of the opposition surge of each surface contain a record of the collisional history of the system. We combine these small phase angle observations with those made at larger phase angles by the New Horizons Long Range Reconnaissance Imager (LORRI), which also has a broadband response with a pivot wavelength of 0.61 microns, to produce the most complete disk-integrated solar phase curves that we will have for decades to come. Modeling these disk-integrated phase curves generates sets of photometric parameters that will inform spectral modeling of the satellite surfaces as well as terrains on Pluto from spatially resolved New Horizons Ralph Linear Etalon Imaging Spectral Array (LEISA) data from 1.2 to 2.5 microns. Rotationally resolved phase curves of Pluto reveal opposition effects that only appear at phase angles less than 0.1 degree and have widths and amplitudes that are highly dependent on longitude and therefore on Pluto's diverse terrains. The high albedo region informally known as Sputnik Planum dominates the disk-integrated reflectance of Pluto on the New Horizons encounter hemisphere. These results lay the groundwork for observations at true opposition in 2018, when the Pluto system will be observable at phase angles so small that an Earth transit across the solar disk will be visible from Pluto and its satellites.
NASA Astrophysics Data System (ADS)
Mayr, Lukas; Rameshan, Raffael; Klötzer, Bernhard; Penner, Simon; Rameshan, Christoph
2014-05-01
An ultra-high vacuum (UHV) setup for "real" and "inverse" model catalyst preparation, depth-resolved near-surface spectroscopic characterization, and quantification of catalytic activity and selectivity under technologically relevant conditions is described. Due to the all-quartz reactor attached directly to the UHV-chamber, transfer of the catalyst for in situ testing without intermediate contact to the ambient is possible. The design of the UHV-compatible re-circulating batch reactor setup allows the study of reaction kinetics under close to technically relevant catalytic conditions up to 1273 K without contact to metallic surfaces except those of the catalyst itself. With the attached differentially pumped exchangeable evaporators and the quartz-microbalance thickness monitoring equipment, a reproducible, versatile, and standardised sample preparation is possible. For three-dimensional near-surface sample characterization, the system is equipped with a hemispherical analyser for X-ray photoelectron spectroscopy (XPS), electron-beam or X-ray-excited Auger-electron spectroscopy, and low-energy ion scattering measurements. Due the dedicated geometry of the X-ray gun (54.7°, "magic angle") and the rotatable sample holder, depth analysis by angle-resolved XPS measurements can be performed. Thus, by the combination of characterisation methods with different information depths, a detailed three-dimensional picture of the electronic and geometric structure of the model catalyst can be obtained. To demonstrate the capability of the described system, comparative results for depth-resolved sample characterization and catalytic testing in methanol steam reforming on PdGa and PdZn near-surface intermetallic phases are shown.
NASA Astrophysics Data System (ADS)
Hell, N.; Beiersdorfer, P.; Magee, E. W.; Brown, G. V.
2016-11-01
We report the calibration of the Orion High-Resolution X-ray (OHREX) imaging crystal spectrometer at the EBIT-I electron beam ion trap at Livermore. Two such instruments, dubbed OHREX-1 and OHREX-2, are fielded for plasma diagnostics at the Orion laser facility in the United Kingdom. The OHREX spectrometer can simultaneously house two spherically bent crystals with a radius of curvature of r = 67.2 cm. The focusing properties of the spectrometer allow both for larger distance to the source due to the increase in collected light and for observation of extended sources. OHREX is designed to cover a 2.5°-3° spectral range at Bragg angles around 51.3°. The typically high resolving powers at these large Bragg angles are ideally suited for line shape diagnostics. For instance, the nominal resolving power of the instrument (>10 000) is much higher than the effective resolving power associated with the Doppler broadening due to the temperature of the trapped ions in EBIT-I. The effective resolving power is only around 3000 at typical EBIT-I conditions, which nevertheless is sufficient to set up and test the instrument's spectral characteristics. We have calibrated the spectral range for a number of crystals using well known reference lines in the first and second order and derived the ion temperatures from these lines. We have also made use of the 50 μm size of the EBIT-I source width to characterize the spatial focusing of the spectrometer.
DOE Office of Scientific and Technical Information (OSTI.GOV)
Hell, N.; Dr. Remeis-Sternwarte and ECAP, Universität Erlangen-Nürnberg, Bamberg 96049; Beiersdorfer, P.
2016-11-15
We report the calibration of the Orion High-Resolution X-ray (OHREX) imaging crystal spectrometer at the EBIT-I electron beam ion trap at Livermore. Two such instruments, dubbed OHREX-1 and OHREX-2, are fielded for plasma diagnostics at the Orion laser facility in the United Kingdom. The OHREX spectrometer can simultaneously house two spherically bent crystals with a radius of curvature of r = 67.2 cm. The focusing properties of the spectrometer allow both for larger distance to the source due to the increase in collected light and for observation of extended sources. OHREX is designed to cover a 2.5°–3° spectral range atmore » Bragg angles around 51.3°. The typically high resolving powers at these large Bragg angles are ideally suited for line shape diagnostics. For instance, the nominal resolving power of the instrument (>10 000) is much higher than the effective resolving power associated with the Doppler broadening due to the temperature of the trapped ions in EBIT-I. The effective resolving power is only around 3000 at typical EBIT-I conditions, which nevertheless is sufficient to set up and test the instrument’s spectral characteristics. We have calibrated the spectral range for a number of crystals using well known reference lines in the first and second order and derived the ion temperatures from these lines. We have also made use of the 50 μm size of the EBIT-I source width to characterize the spatial focusing of the spectrometer.« less
NASA Technical Reports Server (NTRS)
Brown, G. S.; Curry, W. J.
1977-01-01
The statistical error of the pointing angle estimation technique is determined as a function of the effective receiver signal to noise ratio. Other sources of error are addressed and evaluated with inadequate calibration being of major concern. The impact of pointing error on the computation of normalized surface scattering cross section (sigma) from radar and the waveform attitude induced altitude bias is considered and quantitative results are presented. Pointing angle and sigma processing algorithms are presented along with some initial data. The intensive mode clean vs. clutter AGC calibration problem is analytically resolved. The use clutter AGC data in the intensive mode is confirmed as the correct calibration set for the sigma computations.