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Sample records for pure spin states

  1. Pure quantum states of a neutrino with rotating spin in dense magnetized matter

    NASA Astrophysics Data System (ADS)

    Arbuzova, E. V.; Lobanov, A. E.; Murchikova, E. M.

    2010-02-01

    The problem of neutrino spin rotation in dense matter and in strong electromagnetic fields is solved in accordance with the basic principles of quantum mechanics. We obtain a complete system of wave functions for a massive Dirac neutrino with an anomalous magnetic moment which are the eigenfunctions of the kinetic momentum operator and have the form of nonspreading wave packets. These wave functions enable one to consider the states of neutrino with rotating spin as pure quantum states and can be used for calculating probabilities of various processes with the neutrino in the framework of the Furry picture.

  2. Pure valley- and spin-entangled states in a MoS2-based bipolar transistor

    NASA Astrophysics Data System (ADS)

    Bai, Chunxu; Zou, Yonglian; Lou, Wen-Kai; Chang, Kai

    2014-11-01

    In this study, we show that the local Andreev reflection not only can be tuned largely by the type of the normal metal electrode, it also is related to the electrostatic potential in the superconductor region in a MoS2-based n (p ) -type metal/superconductor junction. In a MoS2-based n -type metal/n (p ) -type superconductor/p -type metal (n Sp ) transistor, nonlocal pure valley- and spin-entangled current can be tuned by the length and local gate voltage of a superconductor region. In particular, switching the quasiparticle type in both structures results in a series of intriguing features. Such an effect is not attainable in a graphene-based junction where the electron-hole symmetry enables the symmetry results to be observed. Besides, we have shown that the crossed Andreev reflection exhibits a maximum around ξ /2 instead of the exponential decay behavior in conventional superconductors and a maximum around ξ in the graphene material. The proposed straightforward experimental design and pure valley- and spin-entangled state can pave the way for a wider use in the entanglement based on material group-VI dichalcogenides.

  3. Observation of a single spin by transferring its coherence to a high level macroscopic pure state

    SciTech Connect

    Kawamura, Minaru

    2014-12-04

    We discuss about quantum measurement of a single spin in a superconducting RF resonator, where amplification of coherence of the spin is enabled by transferring its coherence to the harmonic oscillator in an non-coherent state with high energy level. This quantum amplification allows that a single spin can induce macroscopic current to permits observation of a single spin state in the number and phase uncertainty relation.

  4. Quantum well state induced oscillation of pure spin currents in Fe/Au/Pd(001) systems.

    PubMed

    Montoya, Eric; Heinrich, Bret; Girt, Erol

    2014-09-26

    Spin pumping at the ferromagnetic metal (Fe)/normal metal (Au) interface and the subsequent spin transport in Au/Pd heterostructures is studied using ferromagnetic resonance. The spin pumping induced damping in the Fe/Pd structure is greatly suppressed by the addition of a Au spacer layer in the structure Fe/Au/Pd. The rapid decrease in the interface damping with an increasing Au layer thickness does not correspond to an expectation based on a simple spin diffusion theory in the Au layer. It is possible to account for this behavior by introducing a partial reflection of spin current at the Au/Pd interface. Furthermore, oscillations in the amplitude of spin pumping damping are observed in the Fe/Au/Pd structure as a function of Au thickness for thicknesses less than half the electron mean free path of bulk Au. This new effect indicates a formation of quantum well states in the accumulated spin density in the Au spacer that affect the time irreversible process of spin pumping.

  5. Quantum Well State Induced Oscillation of Pure Spin Currents in Fe /Au/Pd(001) Systems

    NASA Astrophysics Data System (ADS)

    Montoya, Eric; Heinrich, Bret; Girt, Erol

    2014-09-01

    Spin pumping at the ferromagnetic metal (Fe)/normal metal (Au) interface and the subsequent spin transport in Au/Pd heterostructures is studied using ferromagnetic resonance. The spin pumping induced damping in the Fe/Pd structure is greatly suppressed by the addition of a Au spacer layer in the structure Fe/Au/Pd. The rapid decrease in the interface damping with an increasing Au layer thickness does not correspond to an expectation based on a simple spin diffusion theory in the Au layer. It is possible to account for this behavior by introducing a partial reflection of spin current at the Au /Pd interface. Furthermore, oscillations in the amplitude of spin pumping damping are observed in the Fe/Au/Pd structure as a function of Au thickness for thicknesses less than half the electron mean free path of bulk Au. This new effect indicates a formation of quantum well states in the accumulated spin density in the Au spacer that affect the time irreversible process of spin pumping.

  6. Quantum spin fluctuations in the bulk insulating state of pure and Fe-doped SmB6

    NASA Astrophysics Data System (ADS)

    Akintola, K.; Pal, A.; Potma, M.; Saha, S. R.; Wang, X. F.; Paglione, J.; Sonier, J. E.

    2017-06-01

    The intermediate-valence compound SmB6 is a well-known Kondo insulator, in which the hybridization of itinerant 5 d electrons with localized 4 f electrons leads to a transition from metallic to insulating behavior at low temperatures. Recent studies suggest that SmB6 is a topological insulator, with topological metallic surface states emerging from a fully insulating hybridized bulk band structure. Here, we locally probe the bulk magnetic properties of pure and 0.5 % Fe-doped SmB6 by muon spin rotation/relaxation methods. Below 6 K, the Fe impurity induces simultaneous changes in the bulk local magnetism and the electrical conductivity. In the low-T insulating bulk state we observe a temperature-independent dynamic relaxation rate indicative of low-lying magnetic excitations driven primarily by quantum fluctuations.

  7. Excitation of coherent propagating spin waves by pure spin currents

    PubMed Central

    Demidov, Vladislav E.; Urazhdin, Sergei; Liu, Ronghua; Divinskiy, Boris; Telegin, Andrey; Demokritov, Sergej O.

    2016-01-01

    Utilization of pure spin currents not accompanied by the flow of electrical charge provides unprecedented opportunities for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. It was recently shown that pure spin currents can be used to excite coherent magnetization dynamics in magnetic nanostructures. However, because of the intrinsic nonlinear self-localization effects, magnetic auto-oscillations in the demonstrated devices were spatially confined, preventing their applications as sources of propagating spin waves in magnonic circuits using these waves as signal carriers. Here, we experimentally demonstrate efficient excitation and directional propagation of coherent spin waves generated by pure spin current. We show that this can be achieved by using the nonlocal spin injection mechanism, which enables flexible design of magnetic nanosystems and allows one to efficiently control their dynamic characteristics. PMID:26818232

  8. Quantumness of spin-1 states

    NASA Astrophysics Data System (ADS)

    Bohnet-Waldraff, Fabian; Braun, D.; Giraud, O.

    2016-01-01

    We investigate quantumness of spin-1 states, defined as the Hilbert-Schmidt distance to the convex hull of spin coherent states. We derive its analytic expression in the case of pure states as a function of the smallest eigenvalue of the Bloch matrix and give explicitly the closest classical state for an arbitrary pure state. Numerical evidence is given that the exact formula for pure states provides an upper bound on the quantumness of mixed states. Due to the connection between quantumness and entanglement we obtain new insights into the geometry of symmetric entangled states.

  9. Direct measurement of the concurrence for two-qubit electron spin entangled pure state based on charge detection

    NASA Astrophysics Data System (ADS)

    Liu, Jiong; Zhou, Lan; Sheng, Yu-Bo

    2015-07-01

    We propose a protocol for directly measuring the concurrence of a two-qubit electronic pure entangled state. To complete this task, we first design a parity-check measurement (PCM) which is constructed by two polarization beam splitters (PBSs) and a charge detector. By using the PCM for three rounds, we can achieve the concurrence by calculating the total probability of picking up the odd parity states from the initial states. Since the conduction electron may be a good candidate for the realization of quantum computation, this protocol may be useful in future solid quantum computation. Project supported by the National Natural Science Foundation of China (Grant Nos. 11474168 and 61401222), the Qing Lan Project in Jiangsu Province, China, and the Priority Academic Development Program of Jiangsu Higher Education Institutions, China.

  10. Reversal and excitations of a nanoscale magnetic domain by sustained pure spin currents

    NASA Astrophysics Data System (ADS)

    Zou, Han; Chen, Shuhan; Ji, Yi

    2012-01-01

    Spin-transfer effects induced by pure spin currents are explored in nonlocal spin valves by using sustained injection currents. Compared to pulsed injection currents used in previous experiments, this approach provides persistent spin-transfer torques and preserves the history of the reversal process. A nanoscale domain in a magnetic wire can be switched reversibly by the sustained pure spin currents. In addition, dips in nonlocal spin signal curves are observed at high magnetic fields for only one polarity of the injection currents. This indicates stable-state magnetization precession around the external field driven by the sustained pure spin currents.

  11. Pure spin current devices based on ferromagnetic topological insulators

    PubMed Central

    Götte, Matthias; Joppe, Michael; Dahm, Thomas

    2016-01-01

    Two-dimensional topological insulators possess two counter propagating edge channels with opposite spin direction. Recent experimental progress allowed to create ferromagnetic topological insulators realizing a quantum anomalous Hall (QAH) state. In the QAH state one of the two edge channels disappears due to the strong ferromagnetic exchange field. We investigate heterostructures of topological insulators and ferromagnetic topological insulators by means of numerical transport calculations. We show that spin current flow in such heterostructures can be controlled with high fidelity. Specifically, we propose spintronic devices that are capable of creating, switching and detecting pure spin currents using the same technology. In these devices electrical currents are directly converted into spin currents, allowing a high conversion efficiency. Energy independent transport properties in combination with large bulk gaps in some topological insulator materials may allow operation even at room temperature. PMID:27782187

  12. Pure spin current devices based on ferromagnetic topological insulators.

    PubMed

    Götte, Matthias; Joppe, Michael; Dahm, Thomas

    2016-10-26

    Two-dimensional topological insulators possess two counter propagating edge channels with opposite spin direction. Recent experimental progress allowed to create ferromagnetic topological insulators realizing a quantum anomalous Hall (QAH) state. In the QAH state one of the two edge channels disappears due to the strong ferromagnetic exchange field. We investigate heterostructures of topological insulators and ferromagnetic topological insulators by means of numerical transport calculations. We show that spin current flow in such heterostructures can be controlled with high fidelity. Specifically, we propose spintronic devices that are capable of creating, switching and detecting pure spin currents using the same technology. In these devices electrical currents are directly converted into spin currents, allowing a high conversion efficiency. Energy independent transport properties in combination with large bulk gaps in some topological insulator materials may allow operation even at room temperature.

  13. Pure spin current induced by adiabatic quantum pumping in zigzag-edged graphene nanoribbons

    SciTech Connect

    Souma, Satofumi Ogawa, Matsuto

    2014-05-05

    We show theoretically that pure spin current can be generated in zigzag edged graphene nanoribbons through the adiabatic pumping by edge selective pumping potentials. The origin of such pure spin current is the spin splitting of the edge localized states, which are oppositely spin polarized at opposite edges. In the proposed device, each edge of the ribbon is covered by two independent time-periodic local gate potentials with a definite phase difference, inducing the edge spin polarized current. When the pumping phase difference is opposite in sign between two edges, the total charge currents is zero and the pure edge spin current is generated.

  14. Pure gauge spin-orbit couplings

    NASA Astrophysics Data System (ADS)

    Shikakhwa, M. S.

    2017-01-01

    Planar systems with a general linear spin-orbit interaction (SOI) that can be cast in the form of a non-Abelian pure gauge field are investigated using the language of non-Abelian gauge field theory. A special class of these fields that, though a 2×2 matrix, are Abelian are seen to emerge and their general form is given. It is shown that the unitary transformation that gauges away these fields induces at the same time a rotation on the wave function about a fixed axis but with a space-dependent angle, both of which being characteristics of the SOI involved. The experimentally important case of equal-strength Rashba and Dresselhaus SOI (R+D SOI) is shown to fall within this special class of Abelian gauge fields, and the phenomenon of persistent spin helix (PSH) that emerges in the presence of this latter SOI in a plane is shown to fit naturally within the general formalism developed. The general formalism is also extended to the case of a particle confined to a ring. It is shown that the Hamiltonian on a ring in the presence of equal-strength R+D SOI is unitarily equivalent to that of a particle subject to only a spin-independent but θ-dependent potential with the unitary transformation relating the two being again the space-dependent rotation operator characteristic of R+D SOI.

  15. Gate-Driven Pure Spin Current in Graphene

    NASA Astrophysics Data System (ADS)

    Lin, Xiaoyang; Su, Li; Si, Zhizhong; Zhang, Youguang; Bournel, Arnaud; Zhang, Yue; Klein, Jacques-Olivier; Fert, Albert; Zhao, Weisheng

    2017-09-01

    The manipulation of spin current is a promising solution for low-power devices beyond CMOS. However, conventional methods, such as spin-transfer torque or spin-orbit torque for magnetic tunnel junctions, suffer from large power consumption due to frequent spin-charge conversions. An important challenge is, thus, to realize long-distance transport of pure spin current, together with efficient manipulation. Here, the mechanism of gate-driven pure spin current in graphene is presented. Such a mechanism relies on the electrical gating of carrier-density-dependent conductivity and spin-diffusion length in graphene. The gate-driven feature is adopted to realize the pure spin-current demultiplexing operation, which enables gate-controllable distribution of the pure spin current into graphene branches. Compared with the Elliott-Yafet spin-relaxation mechanism, the D'yakonov-Perel spin-relaxation mechanism results in more appreciable demultiplexing performance. The feature of the pure spin-current demultiplexing operation will allow a number of logic functions to be cascaded without spin-charge conversions and open a route for future ultra-low-power devices.

  16. Anisotropic Absorption of Pure Spin Currents

    NASA Astrophysics Data System (ADS)

    Baker, A. A.; Figueroa, A. I.; Love, C. J.; Cavill, S. A.; Hesjedal, T.; van der Laan, G.

    2016-01-01

    Spin transfer in magnetic multilayers offers the possibility of ultrafast, low-power device operation. We report a study of spin pumping in spin valves, demonstrating that a strong anisotropy of spin pumping from the source layer can be induced by an angular dependence of the total Gilbert damping parameter, α , in the spin sink layer. Using lab- and synchrotron-based ferromagnetic resonance, we show that an in-plane variation of damping in a crystalline Co50 Fe50 layer leads to an anisotropic α in a polycrystalline Ni81 Fe19 layer. This anisotropy is suppressed above the spin diffusion length in Cr, which is found to be 8 nm, and is independent of static exchange coupling in the spin valve. These results offer a valuable insight into the transmission and absorption of spin currents, and a mechanism by which enhanced spin torques and angular control may be realized for next-generation spintronic devices.

  17. Pure spin current in lateral structures

    NASA Astrophysics Data System (ADS)

    Chen, Shuhan

    Spintronics, a frontier academic research area, is advancing rapidly in recent years. It has been chosen as one of the promising candidates for overcoming the obstacles in continuing the "Moore's Law" of the electronics industry. Spintronics employs both spin and charge degrees of freedom of electrons to reduce energy consumption and increase the flexibility of IC design. To achieve this, it is extremely important to understand the generation, transport, and detection of the spin polarized current (spin current). In this work we use a mesoscopic metallic spintronic structure-nonlocal spin valve (NLSV)-for fundamental studies of spintronics. A nonlocal spin valve consists of two ferromagnetic electrodes (a spin injector and a spin detector) bridged by a non-magnetic spin channel. A thin aluminum oxide barrier (~ 2 - 3 nm) has been shown to effectively enhance the spin injection and detection polarizations. We have studied spin injection and detection in these nanoscale structures. Several topics will be discussed in this work. In Chapter 4 we explore spin transport in NLSVs with Ag channels. Substantial spin signals are observed. The temperature dependence of the spin signals indicates long spin diffusion lengths and low surface spin-flip rate in the mesoscopic Ag channels. Chapter 5 will focus on the asymmetric spin absorption across the low-resistance AlOx barriers in NLSVs. This effect allows for a more simplified and efficient detection scheme for the spin accumulation. Then in Chapter 6 we report a large spin signal owing to a highly resistive break-junction. We have also developed a model to describe the spin-charge coupling effect which enables the large spin signal. In the end, Spin Hall Effect (SHE) is investigated in Chapter 7. A mesoscopic Pt film is utilized to inject a spin accumulation into a mesoscopic Cu channel via the SHE. The spin accumulation in Cu can be detected by the nonlocal method. The reciprocal effect -- the inverse Spin Hall Effect - (i

  18. Pure valley and spin polarization current in ferromagnetic graphene junction

    NASA Astrophysics Data System (ADS)

    Wu, Qing-Ping; Liu, Zheng-Fang; Chen, Ai-Xi; Xiao, Xian-Bo; Miao, Guo-Xing

    2017-02-01

    We investigate the band structure and spin- and valley-dependent transport in ferromagnetic graphene double junctions using the transfer matrix method. The ferromagnetic double junctions include a lateral layout of normal/magnetic vector potential/normal/effective exchange field/normal graphene regions. We find that the strain combined with magnetic vector potentials breaks the valley degeneracy, and the strain combined with the effective exchange field breaks the spin degeneracy, so that there exists a spin- and valley-dependent gap in the ferromagnetic graphene double junctions, which allows only one spin species with special valley characteristics to be transported. Thus, this type of junction can achieve simultaneously pure spin- and pure valley-polarized currents and function as a perfect valley filter and a perfect spin filter. The exact nature of the valley filtering and spin filtering can be tuned by the strain, magnetic barrier, and effective exchange field strength.

  19. Ultrahigh spin thermopower and pure spin current in a single-molecule magnet

    PubMed Central

    Luo, Bo; Liu, Juan; Lü, Jing-Tao; Gao, Jin-Hua; Yao, Kai-Lun

    2014-01-01

    Using the non-equilibrium Green's function (NEGF) formalism within the sequential regime, we studied ultrahigh spin thermopower and pure spin current in single-molecule magnet(SMM), which is attached to nonmagnetic metal wires with spin bias and angle (θ) between the easy axis of SMM and the spin orientation in the electrodes. A pure spin current can be generated by tuning the gate voltage and temperature difference with finite spin bias and the arbitrary angle except of . In the linear regime, large thermopower can be obtained by modifying Vg and the angles (θ). These results are useful in fabricating and advantaging SMM devices based on spin caloritronics. PMID:24549224

  20. Magnetization oscillations and waves driven by pure spin currents

    NASA Astrophysics Data System (ADS)

    Demidov, V. E.; Urazhdin, S.; de Loubens, G.; Klein, O.; Cros, V.; Anane, A.; Demokritov, S. O.

    2017-02-01

    Recent advances in the studies of pure spin currents-flows of angular momentum (spin) not accompanied by the electric currents-have opened new horizons for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. The main advantage of pure spin current, as compared to the spin-polarized electric current, is the possibility to exert spin transfer torque on the magnetization in thin magnetic films without the electrical current flow through the material. In addition to minimizing Joule heating and electromigration effects, this enables the implementation of spin torque devices based on the low-loss insulating magnetic materials, and offers an unprecedented geometric flexibility. Here we review the recent experimental achievements in investigations of magnetization oscillations excited by pure spin currents in different nanomagnetic systems based on metallic and insulating magnetic materials. We discuss the spectral properties of spin-current nano-oscillators, and relate them to the spatial characteristics of the excited dynamic magnetic modes determined by the spatially-resolved measurements. We also show that these systems support locking of the oscillations to external microwave signals, as well as their mutual synchronization, and can be used as efficient nanoscale sources of propagating spin waves.

  1. Pure dephasing of single Mn spin in semiconductor quantum dots

    NASA Astrophysics Data System (ADS)

    Liu, Dingyang; Lai, Wenxi; Yang, Wen

    2017-08-01

    We present comprehensive analytical and numerical studies on the pure dephasing of a single Mn spin in a semiconductor quantum dot due to (i) its sp-d exchange interaction with an electronic environment, and (ii) its hyperfine interaction with the nuclear spin environment. For (i), by modeling the electronic environment by an open two-level system, we provide exact analytical expressions and present detailed analysis for the Mn spin pure dephasing in both the Markovian and non-Markovian regimes. This provides a clear physical picture and a general theoretical framework based on which we estimate the Mn spin pure dephasing due to various fluctuations (such as thermal excitation, optical pumping, tunneling, or electron/hole spin relaxation) of the electronic environment and reveals a series of interesting behaviors, such as thermal, optical, and electrical control of the crossover between the Markov and non-Markov regimes. In particular, we find rapid Mn spin pure dephasing on a nanosecond time scale by the thermal fluctuation and optical pumping, but these mechanisms can be strongly suppressed by shifting the electron envelope function relative to the Mn atom with an external electric field through the quantum-confined Stark effect. The thermal fluctuation mechanism is also exponentially suppressed at low temperature. For (ii), we find that the Mn spin dephasing time is limited by the thermal fluctuation of the nuclear spins to a few microseconds even at low temperature and its value varies from sample to sample, depending on the distribution of spinful isotopes on the nearest-neighbor sites surrounding the substitutional Mn atom. Our findings may be useful to understand and suppress the Mn spin pure dephasing for its applications in quantum information processing.

  2. A measurement of. Delta. sigma. sub L (np), the difference between neutron-proton total cross sections in pure longitudinal spin states

    SciTech Connect

    Beddo, M.E.

    1990-10-01

    A measurement off {Delta}{sigma}{sub L}(np), the difference between neutron-proton total cross sections in pure longitudinal spin states, is described. The results will help determine the isospin-zero (I = 0) scattering amplitudes, which are not well known above laboratory energies of 500 MeV, whereas the isospin-one (I = 1) amplitudes are fairly well-determined to 1 GeV. Data points were taken at the Los Alamos Meson Physics Facility (LAMPF) at Los Alamos, New Mexico, for five neutron beam energies: 484, 568, 634,720 and 788 MeV; they are the first in this energy range. Polarized neutrons were produced by charge-exchange of polarized protons on a liquid deuterium target (LD{sub 2}). Large-volume neutron counters detected the neutrons that passed through a polarized proton target. The counters subtended a range of solid angles large enough to allow extrapolation of the scattered neutrons to 0{degree}. Two modifications to the LAMPF accelerator system which were made for this work are described. They included a beam buncher,'' which modified the normal rf-time structure of the proton beam and allowed for the selection of peak-energy neutrons by time-of-flight means, and a computerized beam steering program, which reduced systematic effects due to beam motion at the LD{sub 2} target. The experimental values of {Delta}{sigma}{sub L}(np) are found to be consistent with other np data, including preliminary data from SIN and Saclay, but not with some results from Argonne which used a polarized proton beam and a polarized deuteron target. The I = 0 component was extracted from {Delta}{sigma}{sub L}(np) using existing pp data (I = 1), with the unexpected result that {Delta}{sigma}{sub L}(I = 0) was found to be essentially identical in shape to {Delta}{sigma}{sub L}(I = 1). The significance of this is not yet understood.

  3. Absolutely classical spin states

    NASA Astrophysics Data System (ADS)

    Bohnet-Waldraff, F.; Giraud, O.; Braun, D.

    2017-01-01

    We introduce the concept of "absolutely classical" spin states, in analogy to absolutely separable states of bipartite quantum systems. Absolutely classical states are states that remain classical (i.e., a convex sum of projectors on coherent states of a spin j ) under any unitary transformation applied to them. We investigate the maximal size of the ball of absolutely classical states centered on the maximally mixed state and derive a lower bound for its radius as a function of the total spin quantum number. We also obtain a numerical estimate of this maximal radius and compare it to the case of absolutely separable states.

  4. Quantum spin liquid states

    NASA Astrophysics Data System (ADS)

    Zhou, Yi; Kanoda, Kazushi; Ng, Tai-Kai

    2017-04-01

    This is an introductory review of the physics of quantum spin liquid states. Quantum magnetism is a rapidly evolving field, and recent developments reveal that the ground states and low-energy physics of frustrated spin systems may develop many exotic behaviors once we leave the regime of semiclassical approaches. The purpose of this article is to introduce these developments. The article begins by explaining how semiclassical approaches fail once quantum mechanics become important and then describe the alternative approaches for addressing the problem. Mainly spin-1 /2 systems are discussed, and most of the time is spent in this article on one particular set of plausible spin liquid states in which spins are represented by fermions. These states are spin-singlet states and may be viewed as an extension of Fermi liquid states to Mott insulators, and they are usually classified in the category of so-called S U (2 ), U (1 ), or Z2 spin liquid states. A review is given of the basic theory regarding these states and the extensions of these states to include the effect of spin-orbit coupling and to higher spin (S >1 /2 ) systems. Two other important approaches with strong influences on the understanding of spin liquid states are also introduced: (i) matrix product states and projected entangled pair states and (ii) the Kitaev honeycomb model. Experimental progress concerning spin liquid states in realistic materials, including anisotropic triangular-lattice systems [κ -(ET )2Cu2(CN )3 and EtMe3Sb [Pd (dmit )2]2 ], kagome-lattice system [ZnCu3(OH )6Cl2 ], and hyperkagome lattice system (Na4 Ir3 O8 ), is reviewed and compared against the corresponding theories.

  5. Mixtures of maximally entangled pure states

    SciTech Connect

    Flores, M.M. Galapon, E.A.

    2016-09-15

    We study the conditions when mixtures of maximally entangled pure states remain entangled. We found that the resulting mixed state remains entangled when the number of entangled pure states to be mixed is less than or equal to the dimension of the pure states. For the latter case of mixing a number of pure states equal to their dimension, we found that the mixed state is entangled provided that the entangled pure states to be mixed are not equally weighted. We also found that one can restrict the set of pure states that one can mix from in order to ensure that the resulting mixed state is genuinely entangled. Also, we demonstrate how these results could be applied as a way to detect entanglement in mixtures of the entangled pure states with noise.

  6. Local symmetry properties of pure three-qubit states

    NASA Astrophysics Data System (ADS)

    Carteret, H. A.; Sudbery, A.

    2000-07-01

    Entanglement types of pure states of three spin-½ particles are classified by means of their stabilizers in the group of local unitary transformations. It is shown that the stabilizer is generically discrete, and that a larger stabilizer indicates a stationary value for some local invariant. We describe all the exceptional states with enlarged stabilizers.

  7. Geometrical control of pure spin current induced domain wall depinning

    NASA Astrophysics Data System (ADS)

    Pfeiffer, A.; Reeve, R. M.; Voto, M.; Savero-Torres, W.; Richter, N.; Vila, L.; Attané, J. P.; Lopez-Diaz, L.; Kläui, Mathias

    2017-03-01

    We investigate the pure spin-current assisted depinning of magnetic domain walls in half ring based Py/Al lateral spin valve structures. Our optimized geometry incorporating a patterned notch in the detector electrode, directly below the Al spin conduit, provides a tailored pinning potential for a transverse domain wall and allows for a precise control over the magnetization configuration and as a result the domain wall pinning. Due to the patterned notch, we are able to study the depinning field as a function of the applied external field for certain applied current densities and observe a clear asymmetry for the two opposite field directions. Micromagnetic simulations show that this can be explained by the asymmetry of the pinning potential. By direct comparison of the calculated efficiencies for different external field and spin current directions, we are able to disentangle the different contributions from the spin transfer torque, Joule heating and the Oersted field. The observed high efficiency of the pure spin current induced spin transfer torque allows for a complete depinning of the domain wall at zero external field for a charge current density of 6\\centerdot {{10}11} A m-2, which is attributed to the optimal control of the position of the domain wall.

  8. Dissipation due to pure spin-current generated by spin pumping

    NASA Astrophysics Data System (ADS)

    Taniguchi, Tomohiro; Saslow, Wayne M.

    2014-12-01

    Based on spin-dependent transport theory and thermodynamics, we develop a generalized theory of the Joule heating in the presence of a spin current. Along with the conventional Joule heating consisting of an electric current and electrochemical potential, it is found that the spin current and spin accumulation give an additional dissipation because the spin-dependent scatterings inside bulk and ferromagnetic/nonmagnetic interface lead to a change of entropy. The theory is applied to investigate the dissipation due to pure spin-current generated by spin pumping across a ferromagnetic/nonmagnetic/ferromagnetic multilayer. The dissipation arises from an interface because the spin pumping is a transfer of both the spin angular momentum and the energy from the ferromagnet to conduction electrons near the interface. It is found that the dissipation is proportional to the enhancement of the Gilbert damping constant by spin pumping.

  9. Generating coherent states of entangled spins

    SciTech Connect

    Yu Hongyi; Luo Yu; Yao Wang

    2011-09-15

    A coherent state of many spins contains quantum entanglement, which increases with a decrease in the collective spin value. We present a scheme to engineer this class of pure state based on incoherent spin pumping with a few collective raising or lowering operators. In a pumping scenario aimed for maximum entanglement, the steady state of N-pumped spin qubits realizes the ideal resource for the 1{yields}(N/2) quantum telecloning. We show how the scheme can be implemented in a realistic system of atomic spin qubits in an optical lattice. Error analysis shows that high-fidelity state engineering is possible for N{approx}O(100) spins in the presence of decoherence. The scheme can also prepare a resource state for the secret sharing protocol and for the construction of the large-scale Affleck-Kennedy-Lieb-Tasaki state.

  10. Hierarchy of Stochastic Pure States for Open Quantum System Dynamics

    NASA Astrophysics Data System (ADS)

    Suess, D.; Eisfeld, A.; Strunz, W. T.

    2014-10-01

    We derive a hierarchy of stochastic evolution equations for pure states (quantum trajectories) for open quantum system dynamics with non-Markovian structured environments. This hierarchy of pure states (HOPS) is generally applicable and provides the exact reduced density operator as an ensemble average over normalized states. The corresponding nonlinear equations are presented. We demonstrate that HOPS provides an efficient theoretical tool and apply it to the spin-boson model, the calculation of absorption spectra of molecular aggregates, and energy transfer in a photosynthetic pigment-protein complex.

  11. Quantifying the coherence of pure quantum states

    NASA Astrophysics Data System (ADS)

    Chen, Jianxin; Grogan, Shane; Johnston, Nathaniel; Li, Chi-Kwong; Plosker, Sarah

    2016-10-01

    In recent years, several measures have been proposed for characterizing the coherence of a given quantum state. We derive several results that illuminate how these measures behave when restricted to pure states. Notably, we present an explicit characterization of the closest incoherent state to a given pure state under the trace distance measure of coherence. We then use this result to show that the states maximizing the trace distance of coherence are exactly the maximally coherent states. We define the trace distance of entanglement and show that it coincides with the trace distance of coherence for pure states. Finally, we give an alternate proof to a recent result that the ℓ1 measure of coherence of a pure state is never smaller than its relative entropy of coherence.

  12. Pure spin current transport in gallium doped zinc oxide

    NASA Astrophysics Data System (ADS)

    Althammer, Matthias; Mukherjee, Joynarayan; Geprägs, Stephan; Goennenwein, Sebastian T. B.; Opel, Matthias; Ramachandra Rao, M. S.; Gross, Rudolf

    2017-01-01

    We study the flow of a pure spin current through zinc oxide by measuring the spin Hall magnetoresistance (SMR) in thin film trilayer samples consisting of bismuth-substituted yttrium iron garnet (Bi:YIG), gallium-doped zinc oxide (Ga:ZnO), and platinum. We investigate the dependence of the SMR magnitude on the thickness of the Ga:ZnO interlayer and compare to a Bi:YIG/Pt bilayer. We find that the SMR magnitude is reduced by almost one order of magnitude upon inserting a Ga:ZnO interlayer and continuously decreases with increasing interlayer thickness. Nevertheless, the SMR stays finite even for a 12 nm thick Ga:ZnO interlayer. These results show that a pure spin current indeed can propagate through a several nm-thick degenerately doped zinc oxide layer. We also observe differences in both the temperature and the field dependence of the SMR when comparing tri- and bilayers. Finally, we compare our data to the predictions of a model based on spin diffusion. This shows that interface resistances play a crucial role for the SMR magnitude in these trilayer structures.

  13. Optimally Squeezed Spin States

    NASA Astrophysics Data System (ADS)

    Rojo, Alberto

    2004-03-01

    We consider optimally spin-squeezed states that maximize the sensitivity of the Ramsey spectroscopy, and for which the signal to noise ratio scales as the number of particles N. Using the variational principle we prove that these states are eigensolutions of the Hamiltonian H(λ)=λ S_z^2-S_x, and that, for large N, the states become equivalent to the quadrature squeezed states of the harmonic oscillator. We present numerical results that illustrate the validity of the equivalence. We also present results of spin squeezing via atom-field interactions within the context of the Tavis-Cummings model. An ensemble of N two-level atoms interacts with a quantized cavity field. For all the atoms initially in their ground states, it is shown that spin squeezing of both the atoms and the field can be achieved provided the initial state of the cavity field has coherence between number states differing by 2. Most of the discussion is restricted to the case of a cavity field initially in a coherent state, but initial squeezed states for the field are also discussed. An analytic solution is found that is valid in the limit that the number of atoms is much greater than unity. References: A. G. Rojo, Phys. Rev A, 68, 013807 (2003); Claudiu Genes, P. R. Berman, and A. G. Rojo Phys. Rev. A 68, 043809 (2003).

  14. Graphical calculus for Gaussian pure states

    SciTech Connect

    Menicucci, Nicolas C.; Flammia, Steven T.; Loock, Peter van

    2011-04-15

    We provide a unified graphical calculus for all Gaussian pure states, including graph transformation rules for all local and semilocal Gaussian unitary operations, as well as local quadrature measurements. We then use this graphical calculus to analyze continuous-variable (CV) cluster states, the essential resource for one-way quantum computing with CV systems. Current graphical approaches to CV cluster states are only valid in the unphysical limit of infinite squeezing, and the associated graph transformation rules only apply when the initial and final states are of this form. Our formalism applies to all Gaussian pure states and subsumes these rules in a natural way. In addition, the term 'CV graph state' currently has several inequivalent definitions in use. Using this formalism we provide a single unifying definition that encompasses all of them. We provide many examples of how the formalism may be used in the context of CV cluster states: defining the 'closest' CV cluster state to a given Gaussian pure state and quantifying the error in the approximation due to finite squeezing; analyzing the optimality of certain methods of generating CV cluster states; drawing connections between this graphical formalism and bosonic Hamiltonians with Gaussian ground states, including those useful for CV one-way quantum computing; and deriving a graphical measure of bipartite entanglement for certain classes of CV cluster states. We mention other possible applications of this formalism and conclude with a brief note on fault tolerance in CV one-way quantum computing.

  15. En Route to Solid State Spin Quantum Computing

    NASA Astrophysics Data System (ADS)

    Mehring, M.; Mende, J.; Scherer, W.

    We present routes to quantum information processing in solids. An introduction to electron and nuclear spins as quantum bits (qubits) is given and basic quantum algorithms are discussed. In particular we focus on the preparation of pseudo pure states and pseudo entangled states in solid systems of combined electron and nuclear spins. As an example we demonstrate the Deutsch algorithm of quantum computing in an S-bus system with one electron spin coupled to a many 19F nuclear spins.

  16. Minimal covariant observables identifying all pure states

    NASA Astrophysics Data System (ADS)

    Carmeli, Claudio; Heinosaari, Teiko; Toigo, Alessandro

    2013-09-01

    It has been recently shown by Heinosaari, Mazzarella and Wolf (2013) [1] that an observable that identifies all pure states of a d-dimensional quantum system has minimally 4d-4 outcomes or slightly less (the exact number depending on d). However, no simple construction of this type of minimal observable is known. We investigate covariant observables that identify all pure states and have minimal number of outcomes. It is shown that the existence of this kind of observables depends on the dimension of the Hilbert space.

  17. Generation and coherent control of pure spin currents via terahertz pulses

    NASA Astrophysics Data System (ADS)

    Schüler, Michael; Berakdar, Jamal

    2014-04-01

    We inspect the time and spin-dependent, inelastic tunneling in engineered semiconductor-based double quantum well driven by time-structured terahertz pulses. An essential ingredient is an embedded spin-active structure with vibrational modes that scatter the pulse driven carriers. Due to the different time scales of the charge and spin dynamics, the spin-dependent electron-vibron coupling may result in pure net spin current (with negligible charge current). Heating the vibrational site may affect the resulting spin current. Furthermore, by controlling the charge dynamics, the spin dynamics and the generated spin current can be manipulated and switched on and off coherently.

  18. Interaction between spin-wave excitations and pure spin currents in magnetic structures

    NASA Astrophysics Data System (ADS)

    Azevedo, Antonio

    2012-02-01

    The generation of pure spin current (PSC) in magnetic structures has attracted much attention not only for its fundamental importance in spintronics, but also because it opens up potential applications. One of the most exciting aspects of this area is the interplay between spin-waves (SW) and PSC. Here we report experimental results in which the PSC, generated by both spin pumping (SPE) [1] and spin Seebeck (SSE) [2] effects, can exert a spin-transfer torque sufficient to compensate the SW relaxation in yttrium iron garnet (YIG)/non-magnetic structures. By measuring the propagation of SW packets in single-crystal YIG films we were able to observe the amplification of volume and magnetostatic modes (MSW) by both SSE and SHE [3,4]. The excitation and detection of the SW packets is carried out by using a MSW delay line device. In both cases the amplification is attributed to the spin-transfer torque due to PSC generated by SSE as well as SHE. It will also be presented new results in which PSC are simultaneously excited by SSE and SPE effects in YIG films. While the spin current generated by SPE is obtained by exciting the ferromagnetic resonance (FMR) of the YIG film, the spin current due to SSE is created by applying a temperature gradient along the film plane. The effect of the superposition of both spin currents is characterized by measuring the spin Hall voltage (VH) along thin strips of Pt deposited on top of the YIG films. Whereas VH corresponding to the uniform FMR is amplified due the SSE the voltages corresponding to the other magnetostatic spin-wave modes are attenuated [5]. [4pt] [1] Y. Tserkovnyak, et al., Rev. Mod. Phys. 77, 1375 (2005).[0pt] [2] K. Uchida, et al., Nature 455, 778 (2008).[0pt] [3] E. Padr'on-Hern'andez, A. Azevedo, and S. M. Rezende, Phys. Rev. Letts., 107, 197203 (2011).[0pt] [4] E. Padr'on-Hern'andez, A. Azevedo, and S. M. Rezende, Appl. Phys. Letts., 99 (2011) in press.[0pt] [5] G.L. da Silva, L.H. Vilela-Leão, S. M. Rezende and A

  19. Voltage-controllable generator of pure spin current: A three-terminal model

    SciTech Connect

    Ma, Zheng; Wu, Reng-Lai; Yu, Ya-Bin Wang, Miao

    2014-07-28

    Three-terminal devices have been frequently proposed to generate the pure spin current. However, the controllability and stability of pure spin current still needs to be improved. In this paper, a three-terminal device, composed of a ferromagnetic metallic lead and two nonmagnetic semiconductor leads coupled with a quantum dot, is employed to study the properties of electron spin transport. The results show that when the external voltage on one of nonmagnetic semiconductor leads is adjusted to a proper range, a pure spin current plateau or a fully spin-polarized current plateau appears in another nonmagnetic semiconductor lead. In a wide range of external voltage, the pure spin current or the spin-polarized current is kept unchanged. Since the change of temperature may considerably influence the spin-polarization of current and is inevitable actually, we studied the corresponding compensation to keep the pure spin current unchanged. Furthermore, the effect of device parameters on the pure spin current is also investigated.

  20. Fock expansion of multimode pure Gaussian states

    SciTech Connect

    Cariolaro, Gianfranco; Pierobon, Gianfranco

    2015-12-15

    The Fock expansion of multimode pure Gaussian states is derived starting from their representation as displaced and squeezed multimode vacuum states. The approach is new and appears to be simpler and more general than previous ones starting from the phase-space representation given by the characteristic or Wigner function. Fock expansion is performed in terms of easily evaluable two-variable Hermite–Kampé de Fériet polynomials. A relatively simple and compact expression for the joint statistical distribution of the photon numbers in the different modes is obtained. In particular, this result enables one to give a simple characterization of separable and entangled states, as shown for two-mode and three-mode Gaussian states.

  1. Boundary conditions and formation of pure spin currents in magnetic field

    NASA Astrophysics Data System (ADS)

    Eliashvili, Merab; Tsitsishvili, George

    2017-09-01

    Schrödinger equation for an electron confined to a two-dimensional strip is considered in the presence of homogeneous orthogonal magnetic field. Since the system has edges, the eigenvalue problem is supplied by the boundary conditions (BC) aimed in preventing the leakage of matter away across the edges. In the case of spinless electrons the Dirichlet and Neumann BC are considered. The Dirichlet BC result in the existence of charge carrying edge states. For the Neumann BC each separate edge comprises two counterflow sub-currents which precisely cancel out each other provided the system is populated by electrons up to certain Fermi level. Cancelation of electric current is a good starting point for developing the spin-effects. In this scope we reconsider the problem for a spinning electron with Rashba coupling. The Neumann BC are replaced by Robin BC. Again, the two counterflow electric sub-currents cancel out each other for a separate edge, while the spin current survives thus modeling what is known as pure spin current - spin flow without charge flow.

  2. Manipulation of pure spin current in ferromagnetic metals independent of magnetization

    NASA Astrophysics Data System (ADS)

    Tian, Dai; Li, Yufan; Qu, D.; Huang, S. Y.; Jin, Xiaofeng; Chien, C. L.

    2016-07-01

    Upon the injection of a pure spin current, a ferromagnet, similar to a nonmagnetic metal, also exhibits inverse spin Hall effect (ISHE). We show in Co/Cu/YIG, where the thin Cu layer allows transmission of spin current from YIG into Co but decouples the two ferromagnets, that the interaction between ISHE and ferromagnetic ordering in Co can be unambiguously investigated. By switching on and off the pure spin current contribution, we demonstrate that the ISHE in Co is independent of the direction of the Co magnetization, which clearly suggests that the ISHE in Co is dominated not by the extrinsic impurity scatterings, but from the intrinsic origin.

  3. Adiabatically twisting a magnetic molecule to generate pure spin currents in graphene

    NASA Astrophysics Data System (ADS)

    Islam, Firoz; Benjamin, Colin

    2016-01-01

    The spin-orbit effect in graphene is too muted to have any observable significance with respect to its application in spintronics. However, graphene technology is too valuable to be rendered impotent to spin transport. In this communication we look at the effect of adiabatically twisting a single-molecule magnet embedded in a graphene monolayer. Surprisingly, we see that pure spin currents (zero charge current) can be generated from the system via quantum pumping. In addition we also see that spin-selective current can be pumped from the system. The pure spin current seen is quite resilient to temperature while disorder has a limited effect. Furthermore, the direction of these spin-pumped currents can be easily and exclusively controlled by the magnetization of the single-molecule magnet, with disorder having no effect on the magnetization control of the pumped spin currents.

  4. Adiabatically twisting a magnetic molecule to generate pure spin currents in graphene.

    PubMed

    Islam, Firoz; Benjamin, Colin

    2016-01-27

    The spin-orbit effect in graphene is too muted to have any observable significance with respect to its application in spintronics. However, graphene technology is too valuable to be rendered impotent to spin transport. In this communication we look at the effect of adiabatically twisting a single-molecule magnet embedded in a graphene monolayer. Surprisingly, we see that pure spin currents (zero charge current) can be generated from the system via quantum pumping. In addition we also see that spin-selective current can be pumped from the system. The pure spin current seen is quite resilient to temperature while disorder has a limited effect. Furthermore, the direction of these spin-pumped currents can be easily and exclusively controlled by the magnetization of the single-molecule magnet, with disorder having no effect on the magnetization control of the pumped spin currents.

  5. Quantum state engineering with spins

    NASA Astrophysics Data System (ADS)

    Heidebrecht, A.; Mende, J.; Mehring, M.

    2006-08-01

    Magnetic resonance methods and in particular Nuclear Magnetic Resonance in the liquid state were the first experimental techniques to implement quantum computing algorithms. The main drawbacks of these methods sofar have been the highly mixed nature of the quantum states and scalability issues. Recently, efforts have been made to address these problems by applying magnetic resonance to solid state systems at lower temperatures. In this contribution, we give an overview of our results on accurately controlling and measuring the quantum state of spin systems in the liquid and in particular in the solid state at low temperatures using Nuclear Magnetic Resonance and Electron Spin Resonance.

  6. Stable pure state quantum tomography from five orthonormal bases

    NASA Astrophysics Data System (ADS)

    Carmeli, Claudio; Heinosaari, Teiko; Kech, Michael; Schultz, Jussi; Toigo, Alessandro

    2016-08-01

    For any finite-dimensional Hilbert space, we construct explicitly five orthonormal bases such that the corresponding measurements allow for efficient tomography of an arbitrary pure quantum state. This means that such measurements can be used to distinguish an arbitrary pure state from any other state, pure or mixed, and the pure state can be reconstructed from the outcome distribution in a feasible way. The set of measurements we construct is independent of the unknown state, and therefore our results provide a fixed scheme for pure state tomography, as opposed to the adaptive (state-dependent) scheme proposed by Goyeneche et al. (Phys. Rev. Lett., 115 (2015) 090401). We show that our scheme is robust with respect to noise, in the sense that any measurement scheme which approximates these measurements well enough is equally suitable for pure state tomography. Finally, we present two convex programs which can be used to reconstruct the unknown pure state from the measurement outcome distributions.

  7. Generation of pure spin currents via spin Seebeck effect in self-biased hexagonal ferrite thin films

    SciTech Connect

    Li, Peng; Ellsworth, David; Chang, Houchen; Janantha, Praveen; Richardson, Daniel; Phillips, Preston; Vijayasarathy, Tarah; Wu, Mingzhong; Shah, Faisal

    2014-12-15

    Light-induced generation of pure spin currents in a Pt(2.5 nm)/BaFe{sub 12}O{sub 19}(1.2 μm)/sapphire(0.5 mm) structure is reported. The BaFe{sub 12}O{sub 19} film had strong in-plane uniaxial anisotropy and was therefore self-biased. Upon exposure to light, a temperature difference (ΔT) was established across the BaFe{sub 12}O{sub 19} thickness that gave rise to a pure spin current in the Pt via the spin Seebeck effect. Via the inverse spin Hall effect, the spin current produced an electric voltage across one of the Pt lateral dimensions. The voltage varied with time in the same manner as ΔT and flipped its sign when the magnetization in BaFe{sub 12}O{sub 19} was reversed.

  8. Optical generation of pure spin currents at the indirect gap of bulk Si

    NASA Astrophysics Data System (ADS)

    Bottegoni, F.; Zucchetti, C.; Ciccacci, F.; Finazzi, M.; Isella, G.

    2017-01-01

    We report on the optical generation of a pure spin current at the indirect gap of bulk Si at room temperature in the photon energy range comprised between 1.2 and 1.8 eV. Spin-polarized electrons are promoted to the Δ-valleys of the Si Brillouin zone by circularly polarized light. The photo-generated spin current is then detected by exploiting a Schottky Pt/Si(001) junction: spin-polarized electrons diffuse toward the Pt/Si interface and enter the Pt layer where the spin current is converted into a transverse electromotive field through the inverse spin-Hall effect (ISHE). The photon energy dependence of the ISHE signal is interpreted in the frame of a one-dimensional spin drift-diffusion model, which allows estimating the electron spin lifetime to be τs=15 ±5 ns.

  9. Degradable quantum channels using pure-state to product-of-pure-state isometries

    NASA Astrophysics Data System (ADS)

    Siddhu, Vikesh; Griffiths, Robert B.

    2016-11-01

    We consider a family of quantum channels characterized by the fact that certain (in general nonorthogonal) pure states at the channel entrance are mapped to (tensor) products of pure states (PPP; hence "pcubed") at the complementary outputs (the main output and the "environment") of the channel. The pcubed construction, a reformulation of the twisted-diagonal procedure by M. M. Wolf and D. Pérez-García [Phys. Rev. A 75, 012303 (2007)], 10.1103/PhysRevA.75.012303, can be used to produce a large class of degradable quantum channels; degradable channels are of interest because their quantum capacities are easy to calculate. Several known types of degradable channels are either pcubed channels, or subchannels (employing a subspace of the channel entrance), or continuous limits of pcubed channels. The pcubed construction also yields channels which are neither degradable nor antidegradable (i.e., the complement of a degradable channel); a particular example of a qutrit channel of this type is studied in some detail. Determining whether a pcubed channel is degradable or antidegradable or neither is quite straightforward given the pure input and output states that characterize the channel. Conjugate degradable pcubed channels are always degradable.

  10. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current

    PubMed Central

    Demidov, V. E.; Evelt, M.; Bessonov, V.; Demokritov, S. O.; Prieto, J. L.; Muñoz, M.; Ben Youssef, J.; Naletov, V. V.; de Loubens, G.; Klein, O.; Collet, M.; Bortolotti, P.; Cros, V.; Anane, A.

    2016-01-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533

  11. Entanglement purification and concentration of electron-spin entangled states using quantum-dot spins in optical microcavities

    SciTech Connect

    Wang Chuan; Zhang Yong; Jin Guangsheng

    2011-09-15

    We present an entanglement purification protocol and an entanglement concentration protocol for electron-spin entangled states, resorting to quantum-dot spin and optical-microcavity-coupled systems. The parity-check gates (PCGs) constructed by the cavity-spin-coupling system provide a different method for the entanglement purification of electron-spin entangled states. This protocol can efficiently purify an electron ensemble in a mixed entangled state. The PCGs can also concentrate electron-spin pairs in less-entangled pure states efficiently. The proposed methods are more flexible as only single-photon detection and single-electron detection are needed.

  12. Entanglement bound for multipartite pure states based on local measurements

    SciTech Connect

    Jiang Lizhen; Chen Xiaoyu; Ye Tianyu

    2011-10-15

    An entanglement bound based on local measurements is introduced for multipartite pure states. It is the upper bound of the geometric measure and the relative entropy of entanglement. It is the lower bound of the minimal-measurement entropy. For pure bipartite states, the bound is equal to the entanglement entropy. The bound is applied to pure tripartite qubit states and the exact tripartite relative entropy of entanglement is obtained for a wide class of states.

  13. Conversion of pure spin current to charge current in amorphous bismuth

    SciTech Connect

    Emoto, H.; Ando, Y.; Shinjo, T.; Shiraishi, M.; Shikoh, E.; Fuseya, Y.

    2014-05-07

    Spin Hall angle and spin diffusion length in amorphous bismuth (Bi) are investigated by using conversion of a pure spin current to a charge current in a spin pumping technique. In Bi/Ni{sub 80}Fe{sub 20}/Si(100) sample, a clear direct current (DC) electromotive force due to the inverse spin Hall effect of the Bi layer is observed at room temperature under a ferromagnetic resonance condition of the Ni{sub 80}Fe{sub 20} layer. From the Bi thickness dependence of the DC electromotive force, the spin Hall angle and the spin diffusion length of the amorphous Bi film are estimated to be 0.02 and 8 nm, respectively.

  14. Typical pure nonequilibrium steady states and irreversibility for quantum transport.

    PubMed

    Monnai, Takaaki; Yuasa, Kazuya

    2016-07-01

    It is known that each single typical pure state in an energy shell of a large isolated quantum system well represents a thermal equilibrium state of the system. We show that such typicality holds also for nonequilibrium steady states (NESS's). We consider a small quantum system coupled to multiple infinite reservoirs. In the long run, the total system reaches a unique NESS. We identify a large Hilbert space from which pure states of the system are to be sampled randomly and show that the typical pure states well describe the NESS. We also point out that the irreversible relaxation to the unique NESS is important to the typicality of the pure NESS's.

  15. Pure circular polarization electroluminescence at room temperature with spin-polarized light-emitting diodes.

    PubMed

    Nishizawa, Nozomi; Nishibayashi, Kazuhiro; Munekata, Hiro

    2017-02-21

    We report the room-temperature electroluminescence (EL) with nearly pure circular polarization (CP) from GaAs-based spin-polarized light-emitting diodes (spin-LEDs). External magnetic fields are not used during device operation. There are two small schemes in the tested spin-LEDs: first, the stripe-laser-like structure that helps intensify the EL light at the cleaved side walls below the spin injector Fe slab, and second, the crystalline AlO x spin-tunnel barrier that ensures electrically stable device operation. The purity of CP is depressively low in the low current density (J) region, whereas it increases steeply and reaches close to the pure CP when J > 100 A/cm(2) There, either right- or left-handed CP component is significantly suppressed depending on the direction of magnetization of the spin injector. Spin-dependent reabsorption, spin-induced birefringence, and optical spin-axis conversion are suggested to account for the observed experimental results.

  16. Pure circular polarization electroluminescence at room temperature with spin-polarized light-emitting diodes

    PubMed Central

    Nishibayashi, Kazuhiro

    2017-01-01

    We report the room-temperature electroluminescence (EL) with nearly pure circular polarization (CP) from GaAs-based spin-polarized light-emitting diodes (spin-LEDs). External magnetic fields are not used during device operation. There are two small schemes in the tested spin-LEDs: first, the stripe-laser-like structure that helps intensify the EL light at the cleaved side walls below the spin injector Fe slab, and second, the crystalline AlOx spin-tunnel barrier that ensures electrically stable device operation. The purity of CP is depressively low in the low current density (J) region, whereas it increases steeply and reaches close to the pure CP when J > 100 A/cm2. There, either right- or left-handed CP component is significantly suppressed depending on the direction of magnetization of the spin injector. Spin-dependent reabsorption, spin-induced birefringence, and optical spin-axis conversion are suggested to account for the observed experimental results. PMID:28174272

  17. Direct Detection of Pure ac Spin Current by X-Ray Pump-Probe Measurements

    NASA Astrophysics Data System (ADS)

    Li, J.; Shelford, L. R.; Shafer, P.; Tan, A.; Deng, J. X.; Keatley, P. S.; Hwang, C.; Arenholz, E.; van der Laan, G.; Hicken, R. J.; Qiu, Z. Q.

    2016-08-01

    Despite recent progress in spin-current research, the detection of spin current has mostly remained indirect. By synchronizing a microwave waveform with synchrotron x-ray pulses, we use the ferromagnetic resonance of the Py (Ni81Fe19 ) layer in a Py /Cu /Cu75Mn25/Cu /Co multilayer to pump a pure ac spin current into the Cu75Mn25 and Co layers, and then directly probe the spin current within the Cu75Mn25 layer and the spin dynamics of the Co layer by x-ray magnetic circular dichroism. This element-resolved pump-probe measurement unambiguously identifies the ac spin current in the Cu75Mn25 layer.

  18. Squeezed spin states: Squeezing the spin uncertainty relations

    NASA Technical Reports Server (NTRS)

    Kitagawa, Masahiro; Ueda, Masahito

    1993-01-01

    The notion of squeezing in spin systems is clarified, and the principle for spin squeezing is shown. Two twisting schemes are proposed as building blocks for spin squeezing and are shown to reduce the standard quantum noise, s/2, of the coherent S-spin state down to the order of S(sup 1/3) and 1/2. Applications to partition noise suppression are briefly discussed.

  19. State diagram of an orthogonal spin transfer spin valve device

    SciTech Connect

    Ye, Li; Wolf, Georg; Pinna, Daniele; Chaves-O'Flynn, Gabriel D.; Kent, Andrew D.

    2015-05-21

    We present the switching characteristics of a spin-transfer device that incorporates a perpendicularly magnetized spin-polarizing layer with an in-plane magnetized free and fixed magnetic layer, known as an orthogonal spin transfer spin valve device. This device shows clear switching between parallel (P) and antiparallel (AP) resistance states and the reverse transition (AP → P) for both current polarities. Further, hysteretic transitions are shown to occur into a state with a resistance intermediate between that of the P and AP states, again for both current polarities. These unusual spin-transfer switching characteristics can be explained within a simple macrospin model that incorporates thermal fluctuations and considers a spin-polarized current that is tilted with respect to the free layer's plane, due to the presence of the spin-transfer torque from the polarizing layer.

  20. Enhancement of Pure Spin Currents in Spin Pumping Y3Fe5O12/Cu/metal Trilayers Through Spin Impedance Matching

    NASA Astrophysics Data System (ADS)

    Hammel, P. Chris; Du, Chunhui; Wang, Hailong; Yang, Fengyuan

    2014-03-01

    Spin pumping, driven thermally as well as by Ferromagnetic Resonance (FMR), is being widely used to generate pure spin currents from ferromagnets (FM) into normal metals (NM). Typically, the NM is chosen to be a spin-sink-Pt, W or Ta, while lighter metals such as Cu are rarely used, except to decouple the FM and spin sink. The efficiency of spin pumping is largely determined by the spin mixing conductance of the FM/NM interface. Here, we report a comparative study of spin pumping in Y3Fe5O12 /Cu/Pt and Y3Fe5O12 /Cu/W trilayers with varying Cu thicknesses. Remarkably, we find that insertion of a Cu interlayer between YIG and W substantially improves (over a factor of 4) the spin current injection into W while similar insertion between YIG and Pt degrades the spin current. This is a consequence of a much improved YIG/Cu spin mixing conductance relative to that for YIG/W. This result shows that high quality multilayer FM/NM heterostructures can enable spin mixing conductances to be engineered to enable optimal spin pumping efficiency. We acknowledge the Center for Emergent Materials at OSU, a NSF MRSEC (DMR-0820414), the DOE through grant DE-FG02-03ER46054, LakeShore Cryotronics and NSL at OSU.

  1. Pure second harmonic current-phase relation in spin-filter Josephson junctions.

    PubMed

    Pal, Avradeep; Barber, Z H; Robinson, J W A; Blamire, M G

    2014-01-01

    Higher harmonics in current-phase relations of Josephson Junctions are predicted to be observed when the first harmonic is suppressed. Conventional theoretical models predict higher harmonics to be extremely sensitive to changes in barrier thickness, temperature, and so on. Here we report experiments with Josephson junctions incorporating a spin-dependent tunnelling barrier, revealing a current-phase relation for highly spin polarized barriers that is purely second harmonic in nature and is insensitive to changes in barrier thickness. This observation implies that the standard theory of Cooper pair transport through tunnelling barriers is not applicable for spin-dependent tunnelling barriers.

  2. Number of spin I states for bosons

    SciTech Connect

    Zhang, L. H.; Zhao, Y. M.; Jia, L. Y.; Arima, A.

    2008-01-15

    We study number of spin I states for bosons in this article. We extend Talmi's recursion formulas for number of states with given spin I to boson systems, and we prove empirical formulas for five bosons by using these recursions. We obtain number of states with given spin I and F spin for three and four bosons by using sum rules of six-j and nine-j symbols. We also present empirical formulas of states for d bosons with given spin I and F=F{sub max}-1 and F{sub max}-2.0.

  3. Single biphoton ququarts as either pure or mixed states

    SciTech Connect

    Fedorov, M. V.; Volkov, P. A.; Mikhailova, J. M.

    2011-09-15

    We analyze features of mixed biphoton polarization states, which arise from pure states of polarization-frequency biphoton ququarts after averaging over frequencies of photons. For mixed states, we find their concurrence C, Schmidt parameter K, degree of polarization P, as well as the von Neumann mutual information I. In some simple cases, we also find the relative entropy S{sub rel} and the degree of classical correlations C{sub cl}. In mixed states, the Schmidt parameter does not characterize the degree of entanglement anymore, as it does in pure states. Nevertheless, the Schmidt parameter remains useful even in the case of mixed states because it remains directly related to the degree of polarization. We compare results occurring in the cases of full pure polarization-frequency states of ququarts and mixed states (averaged over frequencies). Differences between these results can be seen in experiments with and without frequency filters in front of a detector.

  4. All entangled pure states violate a single Bell's inequality.

    PubMed

    Yu, Sixia; Chen, Qing; Zhang, Chengjie; Lai, C H; Oh, C H

    2012-09-21

    We show that a single Bell's inequality with two dichotomic observables for each observer, which originates from Hardy's nonlocality proof without inequalities, is violated by all entangled pure states of a given number of particles, each of which may have a different number of energy levels. Thus Gisin's theorem is proved in its most general form from which it follows that for pure states Bell's nonlocality and quantum entanglement are equivalent.

  5. Decoherence mechanisms of 209Bi donor electron spins in isotopically pure 28Si

    NASA Astrophysics Data System (ADS)

    Wolfowicz, Gary; Simmons, Stephanie; Tyryshkin, Alexei M.; George, Richard E.; Riemann, Helge; Abrosimov, Nikolai V.; Becker, Peter; Pohl, Hans-Joachim; Lyon, Stephen A.; Thewalt, Mike L. W.; Morton, John J. L.

    2012-12-01

    Bismuth (209Bi) is the deepest group V donor in silicon and possesses the most extreme characteristics such as a 9/2 nuclear spin and a 1.5 GHz hyperfine coupling. These lead to several potential advantages for a Si:Bi donor electron spin qubit compared to the more common phosphorus donor. Most previous studies on Si:Bi have been performed using natural silicon where linewidths and electron spin coherence times are limited by the presence of 29Si impurities. Here, we describe electron spin resonance (ESR) and electron nuclear double resonance (ENDOR) studies on 209Bi in isotopically pure 28Si. ESR and ENDOR linewidths, transition probabilities, and coherence times are understood in terms of the spin Hamiltonian parameters showing a dependence on field and mI of the 209Bi nuclear spin. We explore various decoherence mechanisms applicable to the donor electron spin, measuring coherence times up to 700 ms at 1.7 K at X band, comparable with 28Si:P. Importantly, the coherence times we measure follow closely to the calculated field gradients of the transition frequencies (df/dB), providing a strong motivation to explore “clock” transitions where coherence lifetimes could be further enhanced.

  6. Information balance in quantum teleportation with an arbitrary pure state

    SciTech Connect

    Li Li; Chen Zengbing

    2005-07-15

    We study a general teleportation scheme with an arbitrary two-party pure state and derive a tight bound of the teleportation fidelity with a predesigned estimation of the unknown state to be teleported. This bound shows a piecewise balance between information gain and state disturbance. We also explain possible physical significance of the balance.

  7. Spin polarization of the split Kondo state.

    PubMed

    von Bergmann, Kirsten; Ternes, Markus; Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

    2015-02-20

    Spin-resolved scanning tunneling microscopy is employed to quantitatively determine the spin polarization of the magnetic field-split Kondo state. Tunneling conductance spectra of a Kondo-screened magnetic atom are evaluated within a simple model taking into account inelastic tunneling due to spin excitations and two Kondo peaks positioned symmetrically around the Fermi energy. We fit the spin state of the Kondo-screened atom with a spin Hamiltonian independent of the Kondo effect and account for Zeeman splitting of the Kondo peak in the magnetic field. We find that the width and the height of the Kondo peaks scales with the Zeeman energy. Our observations are consistent with full spin polarization of the Kondo peaks, i.e., a majority spin peak below the Fermi energy and a minority spin peak above.

  8. Optical Detection of Nuclear Spin States

    DTIC Science & Technology

    2007-01-31

    the control of a three-qubit solid state NMR quantum information processor. 2 . To explore multi-body spin dynamics and their sensitivity to...journals: 1. Entanglement Assisted Metrology, D. G. Cory, NMR Sensors Conference, Washington DC (2004). 2 . Tutorial on the use of nuclear spins for...between π/ 2 pulses is 30.3µs. Except for very short chains ( 3 -4 spins ), the optimal time between pulses is almost independent of the number of spins

  9. Superadiabatic quantum state transfer in spin chains

    NASA Astrophysics Data System (ADS)

    Agundez, R. R.; Hill, C. D.; Hollenberg, L. C. L.; Rogge, S.; Blaauboer, M.

    2017-01-01

    In this paper we propose a superadiabatic protocol where quantum state transfer can be achieved with arbitrarily high accuracy and minimal control across long spin chains with an odd number of spins. The quantum state transfer protocol only requires the control of the couplings between the qubits on the edge and the spin chain. We predict fidelities above 0.99 for an evolution of nanoseconds using typical spin-exchange coupling values of μ eV . Furthermore, by building a superadiabatic formalism on top of this protocol, we propose an effective superadiabatic protocol that retains the minimal control over the spin chain and further improves the fidelity.

  10. Robust Quantum State Transfer in Random Unpolarized Spin Chains

    NASA Astrophysics Data System (ADS)

    Yao, N. Y.; Jiang, L.; Gorshkov, A. V.; Gong, Z.-X.; Zhai, A.; Duan, L.-M.; Lukin, M. D.

    2011-01-01

    We propose and analyze a new approach for quantum state transfer between remote spin qubits. Specifically, we demonstrate that coherent quantum coupling between remote qubits can be achieved via certain classes of random, unpolarized (infinite temperature) spin chains. Our method is robust to coupling-strength disorder and does not require manipulation or control over individual spins. In principle, it can be used to attain perfect state transfer over an arbitrarily long range via purely Hamiltonian evolution and may be particularly applicable in a solid-state quantum information processor. As an example, we demonstrate that it can be used to attain strong coherent coupling between nitrogen-vacancy centers separated by micrometer distances at room temperature. Realistic imperfections and decoherence effects are analyzed.

  11. Faithful Transfer Arbitrary Pure States with Mixed Resources

    NASA Astrophysics Data System (ADS)

    Luo, Ming-Xing; Li, Lin; Ma, Song-Ya; Chen, Xiu-Bo; Yang, Yi-Xian

    2013-09-01

    In this paper, we show that some special mixed quantum resource experience the same property of pure entanglement such as Bell state for quantum teleportation. It is shown that one mixed state and three bits of classical communication cost can be used to teleport one unknown qubit compared with two bits via pure resources. The schemes are easily implement with model physical techniques. Moreover, these resources are also optimal and typical for faithfully remotely prepare an arbitrary qubit, two-qubit and three-qubit states with mixed quantum resources. Our schemes are completed as same as those with pure quantum entanglement resources except only 1 bit additional classical communication cost required. The success probability is independent of the form of the mixed resources.

  12. A Theoretical Study of Pure and Mixed Spin-Polarized Tritium and Helium Triatomic Systems Using Hyperspherical Coordinates

    NASA Astrophysics Data System (ADS)

    Suno, Hiroya

    2014-04-01

    Pure and mixed spin-polarized tritium () and helium (He) triatomic systems are studied using hyperspherical coordinates. A slow variable discretization approach is adopted to solve the nuclear Schrödinger equation, in which the Schrödinger equation in hyperangular coordinates is solved using basis splines at a series of fixed FEM-DVR hyperradii. By using the best empirical interaction potentials, we study comparatively the bound states of ()3, 4He()2, , 4He3 and in the J Π = 0+ symmetry. The bound state energy levels are calculated for all these molecular species except 4He()2, for which we have found no bound state. The calculated wave functions of these species are found all to exhibit a very large spatial extension, indicating the diffuse nature of these bound states. The molecular structure of these species will also be calculated and analyzed in detail.

  13. Entropy for quantum pure states and quantum H theorem

    NASA Astrophysics Data System (ADS)

    Han, Xizhi; Wu, Biao

    2015-06-01

    We construct a complete set of Wannier functions that are localized at both given positions and momenta. This allows us to introduce the quantum phase space, onto which a quantum pure state can be mapped unitarily. Using its probability distribution in quantum phase space, we define an entropy for a quantum pure state. We prove an inequality regarding the long-time behavior of our entropy's fluctuation. For a typical initial state, this inequality indicates that our entropy can relax dynamically to a maximized value and stay there most of time with small fluctuations. This result echoes the quantum H theorem proved by von Neumann [Zeitschrift für Physik 57, 30 (1929), 10.1007/BF01339852]. Our entropy is different from the standard von Neumann entropy, which is always zero for quantum pure states. According to our definition, a system always has bigger entropy than its subsystem even when the system is described by a pure state. As the construction of the Wannier basis can be implemented numerically, the dynamical evolution of our entropy is illustrated with an example.

  14. Five Measurement Bases Determine Pure Quantum States on Any Dimension.

    PubMed

    Goyeneche, D; Cañas, G; Etcheverry, S; Gómez, E S; Xavier, G B; Lima, G; Delgado, A

    2015-08-28

    A long-standing problem in quantum mechanics is the minimum number of observables required for the characterization of unknown pure quantum states. The solution to this problem is especially important for the developing field of high-dimensional quantum information processing. In this work we demonstrate that any pure d-dimensional state is unambiguously reconstructed by measuring five observables, that is, via projective measurements onto the states of five orthonormal bases. Thus, in our method the total number of different measurement outcomes (5d) scales linearly with d. The state reconstruction is robust against experimental errors and requires simple postprocessing, regardless of d. We experimentally demonstrate the feasibility of our scheme through the reconstruction of eight-dimensional quantum states, encoded in the momentum of single photons.

  15. Control aspects of quantum computing using pure and mixed states.

    PubMed

    Schulte-Herbrüggen, Thomas; Marx, Raimund; Fahmy, Amr; Kauffman, Louis; Lomonaco, Samuel; Khaneja, Navin; Glaser, Steffen J

    2012-10-13

    Steering quantum dynamics such that the target states solve classically hard problems is paramount to quantum simulation and computation. And beyond, quantum control is also essential to pave the way to quantum technologies. Here, important control techniques are reviewed and presented in a unified frame covering quantum computational gate synthesis and spectroscopic state transfer alike. We emphasize that it does not matter whether the quantum states of interest are pure or not. While pure states underly the design of quantum circuits, ensemble mixtures of quantum states can be exploited in a more recent class of algorithms: it is illustrated by characterizing the Jones polynomial in order to distinguish between different (classes of) knots. Further applications include Josephson elements, cavity grids, ion traps and nitrogen vacancy centres in scenarios of closed as well as open quantum systems.

  16. Control aspects of quantum computing using pure and mixed states

    PubMed Central

    Schulte-Herbrüggen, Thomas; Marx, Raimund; Fahmy, Amr; Kauffman, Louis; Lomonaco, Samuel; Khaneja, Navin; Glaser, Steffen J.

    2012-01-01

    Steering quantum dynamics such that the target states solve classically hard problems is paramount to quantum simulation and computation. And beyond, quantum control is also essential to pave the way to quantum technologies. Here, important control techniques are reviewed and presented in a unified frame covering quantum computational gate synthesis and spectroscopic state transfer alike. We emphasize that it does not matter whether the quantum states of interest are pure or not. While pure states underly the design of quantum circuits, ensemble mixtures of quantum states can be exploited in a more recent class of algorithms: it is illustrated by characterizing the Jones polynomial in order to distinguish between different (classes of) knots. Further applications include Josephson elements, cavity grids, ion traps and nitrogen vacancy centres in scenarios of closed as well as open quantum systems. PMID:22946034

  17. Optimal dense coding with arbitrary pure entangled states

    SciTech Connect

    Feng, Yuan; Duan, Runyao; Ji, Zhengfeng

    2006-07-15

    We examine dense coding with an arbitrary pure entangled state sharing between the sender and the receiver. Upper bounds on the average success probability in approximate dense coding and on the probability of conclusive results in unambiguous dense coding are derived. We also construct the optimal protocol which saturates the upper bound in each case.

  18. Purely one-dimensional bands with a giant spin-orbit splitting: Pb nanoribbons on Si(553) surface

    PubMed Central

    Kopciuszyński, Marek; Krawiec, Mariusz; Zdyb, Ryszard; Jałochowski, Mieczysław

    2017-01-01

    We report on a giant Rashba type splitting of metallic bands observed in one-dimensional structures prepared on a vicinal silicon substrate. A single layer of Pb on Si(553) orders this vicinal surface making perfectly regular distribution of monatomic steps. Although there is only one layer of Pb, the system reveals very strong metallic and purely one-dimensional character, which manifests itself in multiple surface state bands crossing the Fermi level in the direction parallel to the step edges and a small band gap in the perpendicular direction. As shown by spin-polarized photoemission and density functional theory calculations these surface state bands are spin-polarized and completely decoupled from the rest of the system. The experimentally observed spin splitting of 0.6 eV at room temperature is the largest found to now in the silicon-based metallic nanostructures, which makes the considered system a promising candidate for application in spintronic devices. PMID:28383078

  19. Pure spin-Hall magnetoresistance in Rh/Y3Fe5O12 hybrid

    PubMed Central

    Shang, T.; Zhan, Q. F.; Ma, L.; Yang, H. L.; Zuo, Z. H.; Xie, Y. L.; Li, H. H.; Liu, L. P.; Wang, B. M.; Wu, Y. H.; Zhang, S.; Li, Run-Wei

    2015-01-01

    We report an investigation of anisotropic magnetoresistance (AMR) and anomalous Hall resistance (AHR) of Rh and Pt thin films sputtered on epitaxial Y3Fe5O12 (YIG) ferromagnetic insulator films. For the Pt/YIG hybrid, large spin-Hall magne toresistance (SMR) along with a sizable conventional anisotropic magnetoresistance (CAMR) and a nontrivial temperature dependence of AHR were observed in the temperature range of 5–300 K. In contrast, a reduced SMR with negligible CAMR and AHR was found in Rh/YIG hybrid. Since CAMR and AHR are characteristics for all ferromagnetic metals, our results suggest that the Pt is likely magnetized by YIG due to the magnetic proximity effect (MPE) while Rh remains free of MPE. Thus the Rh/YIG hybrid could be an ideal model system to explore physics and devices associated with pure spin current. PMID:26639108

  20. Variational Energy Decomposition Analysis of Chemical Bonding. 1. Spin-Pure Analysis of Single Bonds.

    PubMed

    Levine, Daniel S; Horn, Paul R; Mao, Yuezhi; Head-Gordon, Martin

    2016-10-11

    We have designed an energy decomposition analysis (EDA) to gain a deeper understanding of single chemical bonds, that is, those in which the interacting fragments are doublet open-shell systems but the supersystem is closed-shell. The method is a spin-pure extension of the absolutely localized molecular orbital (ALMO) EDA to the one-pair perfect pairing energy (equivalently to an active space of two electrons in two orbitals). The total interaction energy is broken up into four terms: frozen interactions, spin-coupling, polarization, and charge-transfer. A variety of single bonds are analyzed and, in addition, we use this method to show how solvation changes the nature of bonds, producing different results in the gas-phase and with explicit solvent molecules.

  1. Molecular dynamics simulations of spin and pure liquids with preservation of all the conservation laws.

    PubMed

    Omelyan, I P; Mryglod, I M; Folk, R

    2001-07-01

    A methodology is developed to integrate numerically the equations of motion for classical many-body systems in molecular dynamics simulations. Its distinguishable feature is the possibility to preserve, independently on the size of the time step, all the conservation laws inherent in the description without breaking the time reversibility. As a result, an implicit second-order algorithm is derived and applied to pure liquids, as well as spin liquids, for which the dynamics is characterized by the conservation of total energy, linear and angular momenta, as well as magnetization and individual spin lengths. It is demonstrated on the basis of Lennard-Jones and Heisenberg fluid models that when such quantities as energy and magnetization must be conserved perfectly, the algorithm turns out to be more efficient than popular decomposition integrators and standard predictor-corrector schemes.

  2. Generating non-classical states from spin coherent states via interaction with ancillary spins

    NASA Astrophysics Data System (ADS)

    Dooley, Shane; Joo, Jaewoo; Proctor, Timothy; Spiller, Timothy P.

    2015-02-01

    The generation of non-classical states of large quantum systems has attracted much interest from a foundational perspective, but also because of the significant potential of such states in emerging quantum technologies. In this paper we consider the possibility of generating non-classical states of a system of spins by interaction with an ancillary system, starting from an easily prepared initial state. We extend previous results for an ancillary system comprising a single spin to bigger ancillary systems and the interaction strength is enhanced by a factor of the number of ancillary spins. Depending on initial conditions, we find - by a combination of approximation and numerics - that the system of spins can evolve to spin cat states, spin squeezed states or to multiple cat states. We also discuss some candidate systems for implementation of the Hamiltonian necessary to generate these non-classical states.

  3. Probabilistically Perfect Cloning of Two Pure States: Geometric Approach

    NASA Astrophysics Data System (ADS)

    Yerokhin, V.; Shehu, A.; Feldman, E.; Bagan, E.; Bergou, J. A.

    2016-05-01

    We solve the long-standing problem of making n perfect clones from m copies of one of two known pure states with minimum failure probability in the general case where the known states have arbitrary a priori probabilities. The solution emerges from a geometric formulation of the problem. This formulation reveals that cloning converges to state discrimination followed by state preparation as the number of clones goes to infinity. The convergence exhibits a phenomenon analogous to a second-order symmetry-breaking phase transition.

  4. Spin state switching in iron coordination compounds

    PubMed Central

    Gaspar, Ana B; Garcia, Yann

    2013-01-01

    Summary The article deals with coordination compounds of iron(II) that may exhibit thermally induced spin transition, known as spin crossover, depending on the nature of the coordinating ligand sphere. Spin transition in such compounds also occurs under pressure and irradiation with light. The spin states involved have different magnetic and optical properties suitable for their detection and characterization. Spin crossover compounds, though known for more than eight decades, have become most attractive in recent years and are extensively studied by chemists and physicists. The switching properties make such materials potential candidates for practical applications in thermal and pressure sensors as well as optical devices. The article begins with a brief description of the principle of molecular spin state switching using simple concepts of ligand field theory. Conditions to be fulfilled in order to observe spin crossover will be explained and general remarks regarding the chemical nature that is important for the occurrence of spin crossover will be made. A subsequent section describes the molecular consequences of spin crossover and the variety of physical techniques usually applied for their characterization. The effects of light irradiation (LIESST) and application of pressure are subjects of two separate sections. The major part of this account concentrates on selected spin crossover compounds of iron(II), with particular emphasis on the chemical and physical influences on the spin crossover behavior. The vast variety of compounds exhibiting this fascinating switching phenomenon encompasses mono-, oligo- and polynuclear iron(II) complexes and cages, polymeric 1D, 2D and 3D systems, nanomaterials, and polyfunctional materials that combine spin crossover with another physical or chemical property. PMID:23504535

  5. Experimentally superposing two pure states with partial prior knowledge

    NASA Astrophysics Data System (ADS)

    Li, Keren; Long, Guofei; Katiyar, Hemant; Xin, Tao; Feng, Guanru; Lu, Dawei; Laflamme, Raymond

    2017-02-01

    Superposition, arguably the most fundamental property of quantum mechanics, lies at the heart of quantum information science. However, how to create the superposition of any two unknown pure states remains as a daunting challenge. Recently, it was proved that such a quantum protocol does not exist if the two input states are completely unknown, whereas a probabilistic protocol is still available with some prior knowledge about the input states [M. Oszmaniec et al., Phys. Rev. Lett. 116, 110403 (2016), 10.1103/PhysRevLett.116.110403]. The knowledge is that both of the two input states have nonzero overlaps with some given referential state. In this work, we experimentally realize the probabilistic protocol of superposing two pure states in a three-qubit nuclear magnetic resonance system. We demonstrate the feasibility of the protocol by preparing a families of input states, and the average fidelity between the prepared state and expected superposition state is over 99%. Moreover, we experimentally illustrate the limitation of the protocol that it is likely to fail or yields very low fidelity, if the nonzero overlaps are approaching zero. Our experimental implementation can be extended to more complex situations and other quantum systems.

  6. Classical-hidden-variable description for entanglement dynamics of two-qubit pure states

    NASA Astrophysics Data System (ADS)

    Silveira, L. S.; Angelo, R. M.

    2017-06-01

    A hidden-variable model is explicitly constructed by use of a Liouvillian description for the dynamics of two coupled spin-1/2 particles. In this model, the underlying Hamiltonian trajectories play the role of deterministic hidden variables, whereas the shape of the initial probability distribution figures as a hidden variable that regulates the capacity of the model in producing correlations. We show that even though the model can very well describe the short-time entanglement dynamics of initially separated pure states, it is incapable of violating the Clauser-Horne-Shimony-Holt inequality. Our work suggests that, if one takes the reluctance of a given quantum resource to be emulated by a local-hidden-variable model as a signature of its nonclassicality degree, then one can conclude that entanglement and nonlocality are nonequivalent even in the context of two-qubit pure states.

  7. Spin flip of multiqubit states in discrete phase space

    NASA Astrophysics Data System (ADS)

    Srinivasan, K.; Raghavan, G.

    2017-02-01

    Time reversal and spin flip are discrete symmetry operations of substantial importance to quantum information and quantum computation. Spin flip arises in the context of separability, quantification of entanglement and the construction of universal NOT gates. The present work investigates the relationship between the quantum state of a multiqubit system represented by the discrete Wigner function (DWFs) and its spin-flipped counterpart. The two are shown to be related through a Hadamard matrix that is independent of the choice of the quantum net used for the tomographic reconstruction of the DWF. These results are of interest to cases involving the direct tomographic reconstruction of the DWF from experimental data, and in the analysis of entanglement related properties purely in terms of the DWF.

  8. Purely optical navigation with model-based state prediction

    NASA Astrophysics Data System (ADS)

    Sendobry, Alexander; Graber, Thorsten; Klingauf, Uwe

    2010-10-01

    State-of-the-art Inertial Navigation Systems (INS) based on Micro-Electro-Mechanical Systems (MEMS) have a lack of precision especially in GPS denied environments like urban canyons or in pure indoor missions. The proposed Optical Navigation System (ONS) provides bias free ego-motion estimates using triple redundant sensor information. In combination with a model based state prediction our system is able to estimate velocity, position and attitude of an arbitrary aircraft. Simulating a high performance flow-field estimator the algorithm can compete with conventional low-cost INS. By using measured velocities instead of accelerations the system states drift behavior is not as distinctive as for an INS.

  9. Observation of pure inverse spin Hall effect in ferromagnetic metals via ferromagnetic/antiferromagnetic exchange-bias structures

    NASA Astrophysics Data System (ADS)

    Wu, H.; Wan, C. H.; Yuan, Z. H.; Zhang, X.; Jiang, J.; Zhang, Q. T.; Wen, Z. C.; Han, X. F.

    2015-08-01

    We report that the spin current generated by the spin Seebeck effect (SSE) in yttrium iron garnet (YIG) can be detected by a ferromagnetic metal (NiFe). By using the ferromagnetic/antiferromagnetic (FM/AFM) exchange bias structure (NiFe/IrMn), the inverse spin Hall effect (ISHE) and planar Nernst effect (PNE) of NiFe can be unambiguously separated, allowing us to observe a pure ISHE signal. After eliminating the in-plane temperature gradient in NiFe, we can even observe a pure ISHE signal without PNE from NiFe itself. It is worth noting that a large spin Hall angle (0.098) of NiFe is obtained, which is comparable with Pt. This work provides a kind of FM/AFM exchange bias structure to detect the spin current by charge signals, and highlights that ISHE in ferromagnetic metals can be used in spintronic research and applications.

  10. All pure bipartite entangled states can be self-tested

    NASA Astrophysics Data System (ADS)

    Coladangelo, Andrea; Goh, Koon Tong; Scarani, Valerio

    2017-05-01

    Quantum technologies promise advantages over their classical counterparts in the fields of computation, security and sensing. It is thus desirable that classical users are able to obtain guarantees on quantum devices, even without any knowledge of their inner workings. That such classical certification is possible at all is remarkable: it is a consequence of the violation of Bell inequalities by entangled quantum systems. Device-independent self-testing refers to the most complete such certification: it enables a classical user to uniquely identify the quantum state shared by uncharacterized devices by simply inspecting the correlations of measurement outcomes. Self-testing was first demonstrated for the singlet state and a few other examples of self-testable states were reported in recent years. Here, we address the long-standing open question of whether every pure bipartite entangled state is self-testable. We answer it affirmatively by providing explicit self-testing correlations for all such states.

  11. Cooperative pulses for pseudo-pure state preparation

    SciTech Connect

    Wei, Daxiu; Chang, Yan; Yang, Xiaodong E-mail: xiaodong.yang@sibet.ac.cn; Glaser, Steffen J. E-mail: xiaodong.yang@sibet.ac.cn

    2014-06-16

    Using an extended version of the optimal-control-based gradient ascent pulse engineering algorithm, cooperative (COOP) pulses are designed for multi-scan experiments to prepare pseudo-pure states in quantum computation. COOP pulses can cancel undesired signal contributions, complementing and generalizing phase cycles. They also provide more flexibility and, in particular, eliminate the need to select specific individual target states and achieve the fidelity of theoretical limit by flexibly choosing appropriate number of scans and duration of pulses. The COOP approach is experimentally demonstrated for three-qubit and four-qubit systems.

  12. Optimal cloning of pure states, testing single clones

    NASA Astrophysics Data System (ADS)

    Keyl, M.; Werner, R. F.

    1999-07-01

    We consider quantum devices for turning a finite number N of d-level quantum systems in the same unknown pure state σ into M>N systems of the same kind, in an approximation of the M-fold tensor product of the state σ. In a previous paper it was shown that this problem has a unique optimal solution, when the quality of the output is judged by arbitrary measurements, involving also the correlations between the clones. We show in this paper, that if the quality judgment is based solely on measurements of single output clones, there is again a unique optimal cloning device, which coincides with the one found previously.

  13. High-spin states of ZXRh

    SciTech Connect

    Piel W.F. Jr.; Scharff-Goldhaber, G.; Lister, C.J.; Varley, B.J.

    1986-02-01

    High-spin states of ZXRh up to J = ((31/2)) and an excitation energy of 7.1 MeV were established by means of the WNi(UCa,3pel)ZXRh reaction. The states are found to decay through two separate el-ray cascades with the assignments for the lower-spin states being in agreement with previous work. No strong evidence has been found for the existence of collectivity induced by intruder states. The empirical excitation energies are compared to those found recently for the nearby even-A isotones ZWRu and ZYPd, and the systematics of the N = 52 nuclides are discussed.

  14. All entangled pure quantum states violate the bilocality inequality

    NASA Astrophysics Data System (ADS)

    Gisin, Nicolas; Mei, Quanxin; Tavakoli, Armin; Renou, Marc Olivier; Brunner, Nicolas

    2017-08-01

    The nature of quantum correlations in networks featuring independent sources of entanglement remains poorly understood. Here, focusing on the simplest network of entanglement swapping, we start a systematic characterization of the set of quantum states leading to violation of the so-called "bilocality" inequality. First, we show that all possible pairs of entangled pure states can violate the inequality. Next, we derive a general criterion for violation for arbitrary pairs of mixed two-qubit states. Notably, this reveals a strong connection between the Clauser-Horne-Shimony-Holt (CHSH) Bell inequality and the bilocality inequality, namely, that any entangled state violating CHSH also violates the bilocality inequality. We conclude with a list of open questions.

  15. Slow spin dynamics between ferromagnetic chains in a pure-inorganic framework.

    PubMed

    David, Rénald; Kabbour, Houria; Colis, Silviu; Mentré, Olivier

    2013-12-02

    The crystal structure of the new phase BaCo(II)2(As(III)3O6)2·2(H2O) is built from the stacking of infinite [BaCo2(As3O6)2·H2O] sheets containing ∞[Co(II)O4](6-) chains interconnected by perpendicular ∞[As(III)O2](-) chains. It shows a metamagnetic transition below ∼9 K at a critical field of ∼0.11 T, leading to a moment value of 70% of the expected saturation, related to the spin flip between individual robust canted ferromagnetic chains. We propose a field-dependent scenario with magnetic moments lying in the Co(II)O6 octahedral basal planes, fully compatible with our experimental results. Magnetic measurements under ac-field show slow spin dynamics with an intrinsic single-chain magnet (SCM)-like component slightly modified in the field-aligned regime. The characteristic relaxation time and energy barrier are about τo = 5.1 × 10(-10) s and Δτ = 35.3 K at H(dc) = 0, respectively, which falls close to values found for other (but organometallic) SCM Co(II) chains. This magnetic behavior is unique in the field of pure-inorganic compounds.

  16. Regression relation for pure quantum states and its implications for efficient computing.

    PubMed

    Elsayed, Tarek A; Fine, Boris V

    2013-02-15

    We obtain a modified version of the Onsager regression relation for the expectation values of quantum-mechanical operators in pure quantum states of isolated many-body quantum systems. We use the insights gained from this relation to show that high-temperature time correlation functions in many-body quantum systems can be controllably computed without complete diagonalization of the Hamiltonians, using instead the direct integration of the Schrödinger equation for randomly sampled pure states. This method is also applicable to quantum quenches and other situations describable by time-dependent many-body Hamiltonians. The method implies exponential reduction of the computer memory requirement in comparison with the complete diagonalization. We illustrate the method by numerically computing infinite-temperature correlation functions for translationally invariant Heisenberg chains of up to 29 spins 1/2. Thereby, we also test the spin diffusion hypothesis and find it in a satisfactory agreement with the numerical results. Both the derivation of the modified regression relation and the justification of the computational method are based on the notion of quantum typicality.

  17. Chimera states in purely local delay-coupled oscillators.

    PubMed

    Bera, Bidesh K; Ghosh, Dibakar

    2016-05-01

    We study the existence of chimera states in a network of locally coupled chaotic and limit-cycle oscillators. The necessary condition for chimera state in purely local coupled oscillators is discussed. At first, we numerically observe the existence of chimera or multichimera states in the locally coupled Hindmarsh-Rose neuron model. We find that delay time in the nonlinear local coupling reduces the domain of the coherent island in the parameter space of the synaptic coupling strength and time delay, and thus the coherent region can be completely eliminated once the time delay exceeds a certain threshold. We then consider another form of nonlinearity in the local coupling, and the existence of chimera states is observed in the time-delayed Mackey-Glass system and in a Van der Pol oscillator. We also discuss the effect of time delay in local coupling for the existence of chimera states in Mackey-Glass systems. The nonlinearity present in the coupling function plays a key role in the emergence of chimera or multichimera states. A phase diagram for the chimera state is identified over a wide parameter space.

  18. Chimera states in purely local delay-coupled oscillators

    NASA Astrophysics Data System (ADS)

    Bera, Bidesh K.; Ghosh, Dibakar

    2016-05-01

    We study the existence of chimera states in a network of locally coupled chaotic and limit-cycle oscillators. The necessary condition for chimera state in purely local coupled oscillators is discussed. At first, we numerically observe the existence of chimera or multichimera states in the locally coupled Hindmarsh-Rose neuron model. We find that delay time in the nonlinear local coupling reduces the domain of the coherent island in the parameter space of the synaptic coupling strength and time delay, and thus the coherent region can be completely eliminated once the time delay exceeds a certain threshold. We then consider another form of nonlinearity in the local coupling, and the existence of chimera states is observed in the time-delayed Mackey-Glass system and in a Van der Pol oscillator. We also discuss the effect of time delay in local coupling for the existence of chimera states in Mackey-Glass systems. The nonlinearity present in the coupling function plays a key role in the emergence of chimera or multichimera states. A phase diagram for the chimera state is identified over a wide parameter space.

  19. Higher spin states in neutron rich nuclei

    NASA Astrophysics Data System (ADS)

    Zhu, S.; Zhao, X.; Hamilton, J. H.; Ramayya, A. V.; Ma, W. C.; Peker, L. K.; Kormicki, J.; Hong, X.; Gao, W. B.; Deng, J. K.

    Nuclei on the neutron rich side of beta stability have long been of interest for nuclear structure studies because they probe different regions of the single particle spectrum and different shell gap combinations for both spherical and deformed shapes. However, such nuclei have been a difficult challenge experimentally. Much information has been gained about the properties of neutron rich nuclei at low spin from the study of radioactive isotopes produced in neutron induced, and more recently, proton induced fission of uranium. Such studies have been made possible by the use of isotope separators on line to reactors and more recently to low energy proton accelerators. However, to test many of the theoretical predictions of nuclear models one needs information about the higher spin states in nuclei in addition to their low spin states populated in radioactive decays. Higher spin states in neutron rich nuclei have been an even more difficult challenge than the lower spin states accessible through decay studies. One cannot reach the higher spin states in these nuclei by heavy ion fusion evaporation in reactions as carried out extensively for proton rich nuclei. Many years ago prompt spontaneous fission studies were used to suggest for the first time that Sr-98 and Zr-100 had unusually large ground state of deformations. The availability of higher efficiency multi-detector arrays of Compton suppressed Ge detectors has brought on a renewed interest in studies of the prompt gamma rays of the fragments from spontaneous and induced fission. Groups at Argonne, Daresbury, and a Vanderbilt-Oak Ridge-Idaho-Dubna collaboration have carried out several such studies from spontaneous and heavy-ion induced fission which have revealed new insights into our knowledge of neutron rich nuclei. This paper is primarily a review of these studies, including recent, unpublished results.

  20. Generating quantum states through spin chain dynamics

    NASA Astrophysics Data System (ADS)

    Kay, Alastair

    2017-04-01

    The spin chain is a theoretical work-horse of the physicist, providing a convenient, tractable model that yields insight into a host of physical phenomena including conduction, frustration, superconductivity, topological phases, localisation, phase transitions, quantum chaos and even string theory. Our ultimate aim, however, is not just to understand the properties of a physical system, but to harness it for our own ends. We therefore study the possibilities for engineering a special class of spin chain, envisaging the potential for this to feedback into the original physical systems. We pay particular attention to the generation of multipartite entangled states such as the W (Dicke) state, superposed over multiple sites of the chain.

  1. Topologically protected localised states in spin chains

    PubMed Central

    Estarellas, Marta P.; D’Amico, Irene; Spiller, Timothy P.

    2017-01-01

    We consider spin chain families inspired by the Su, Schrieffer and Hegger (SSH) model. We demonstrate explicitly the topologically induced spatial localisation of quantum states in our systems. We present detailed investigations of the effects of random noise, showing that these topologically protected states are very robust against this type of perturbation. Systems with such topological robustness are clearly good candidates for quantum information tasks and we discuss some potential applications. Thus, we present interesting spin chain models which show promising applications for quantum devices. PMID:28225002

  2. Topologically protected localised states in spin chains

    NASA Astrophysics Data System (ADS)

    Estarellas, Marta P.; D’Amico, Irene; Spiller, Timothy P.

    2017-02-01

    We consider spin chain families inspired by the Su, Schrieffer and Hegger (SSH) model. We demonstrate explicitly the topologically induced spatial localisation of quantum states in our systems. We present detailed investigations of the effects of random noise, showing that these topologically protected states are very robust against this type of perturbation. Systems with such topological robustness are clearly good candidates for quantum information tasks and we discuss some potential applications. Thus, we present interesting spin chain models which show promising applications for quantum devices.

  3. Passive interferometric symmetries of multimode Gaussian pure states

    NASA Astrophysics Data System (ADS)

    Gabay, Natasha; Menicucci, Nicolas C.

    2016-05-01

    As large-scale multimode Gaussian states begin to become accessible in the laboratory, their representation and analysis become a useful topic of research in their own right. The graphical calculus for Gaussian pure states provides powerful tools for their representation, while this work presents a useful tool for their analysis: passive interferometric (i.e., number-conserving) symmetries. Here we show that these symmetries of multimode Gaussian states simplify calculations in measurement-based quantum computing and provide constructive tools for engineering large-scale harmonic systems with specific physical properties, and we provide a general mathematical framework for deriving them. Such symmetries are generated by linear combinations of operators expressed in the Schwinger representation of U (2 ) , called nullifiers because the Gaussian state in question is a zero eigenstate of them. This general framework is shown to have applications in the noise analysis of continuous-various cluster states and is expected to have additional applications in future work with large-scale multimode Gaussian states.

  4. Monogamy of quantum correlations in three-qubit pure states

    NASA Astrophysics Data System (ADS)

    Sudha; Devi, A. R. Usha; Rajagopal, A. K.

    2012-01-01

    The limitation on the shareability of quantum entanglement over several parties, the so-called monogamy of entanglement, is an issue that has received considerable attention from the quantum information community over the last decade. A natural question of interest in this connection is whether monogamy of correlations is true for correlations other than entanglement. This issue is examined here by choosing quantum deficit, proposed by A. K. Rajagopal and R. W. Rendell [Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.66.022104 66, 022104 (2002)], an operational measure of correlations. In addition to establishing the polygamous nature of the class of three-qubit symmetric pure states characterized by two distinct Majorana spinors (to which the W states belong), those with three distinct Majorana spinors [to which Greenberger-Horne-Zeilinger (GHZ) states belong] are shown to either obey or violate monogamy relations. While the generalized W states can be monogamous or polygamous, the generalized GHZ states exhibit monogamy with respect to quantum deficit. The issue of using monogamy conditions based on quantum deficit to witness the states belonging to stochastic local operations and classical communication (SLOCC) inequivalent classes is discussed in light of these results.

  5. Distribution of G concurrence of random pure states

    SciTech Connect

    Cappellini, Valerio; Zyczkowski, Karol

    2006-12-15

    The average entanglement of random pure states of an NxN composite system is analyzed. We compute the average value of the determinant D of the reduced state, which forms an entanglement monotone. Calculating higher moments of the determinant, we characterize the probability distribution P(D). Similar results are obtained for the rescaled Nth root of the determinant, called the G concurrence. We show that in the limit N{yields}{infinity} this quantity becomes concentrated at a single point G{sub *}=1/e. The position of the concentration point changes if one consider an arbitrary NxK bipartite system, in the joint limit N,K{yields}{infinity}, with K/N fixed.

  6. Fluctuation Theorem for Many-Body Pure Quantum States

    NASA Astrophysics Data System (ADS)

    Iyoda, Eiki; Kaneko, Kazuya; Sagawa, Takahiro

    2017-09-01

    We prove the second law of thermodynamics and the nonequilibrium fluctuation theorem for pure quantum states. The entire system obeys reversible unitary dynamics, where the initial state of the heat bath is not the canonical distribution but is a single energy eigenstate that satisfies the eigenstate-thermalization hypothesis. Our result is mathematically rigorous and based on the Lieb-Robinson bound, which gives the upper bound of the velocity of information propagation in many-body quantum systems. The entanglement entropy of a subsystem is shown connected to thermodynamic heat, highlighting the foundation of the information-thermodynamics link. We confirmed our theory by numerical simulation of hard-core bosons, and observed dynamical crossover from thermal fluctuations to bare quantum fluctuations. Our result reveals a universal scenario that the second law emerges from quantum mechanics, and can be experimentally tested by artificial isolated quantum systems such as ultracold atoms.

  7. Timekeeping with electron spin states in diamond

    NASA Astrophysics Data System (ADS)

    Hodges, J. S.; Yao, N. Y.; Maclaurin, D.; Rastogi, C.; Lukin, M. D.; Englund, D.

    2013-03-01

    Frequency standards based on atomic states, such as Rb or Cs vapors, or single-trapped ions, are the most precise measures of time. Here we propose and analyze a precision oscillator approach based upon spins in a solid-state system, in particular, the nitrogen-vacancy defect in single-crystal diamond. We show that this system can have stability approaching portable atomic standards and is readily incorporable as a chip-scale device. Using a pulsed spin-echo technique, we anticipate an Allan deviation of σy=10-7τ-1/2 limited by thermally-induced strain variations; in the absence of such thermal fluctuations, the system is limited by spin dephasing and harbors an Allan deviation nearing ˜10-12τ-1/2. Potential improvements based upon advanced diamond material processing, temperature stabilization, and nanophotonic engineering are discussed.

  8. Quantum entanglement swapping of two arbitrary biqubit pure states

    NASA Astrophysics Data System (ADS)

    Xie, ChuanMei; Liu, YiMin; Chen, JianLan; Yin, XiaoFeng; Zhang, ZhanJun

    2016-10-01

    In this paper, the issue of swapping quantum entanglements in two arbitrary biqubit pure states via a local bipartite entangledstate projective measure in the middle node is studied in depth, especially with regard to quantitative aspects. Attention is mainly focused on the relation between the measure and the final entanglement obtained via swapping. During the study, the entanglement of formation (EoF) is employed as a quantifier to characterize and quantify the entanglements present in all involved states. All concerned EoFs are expressed analytically; thus, the relation between the final entanglement and the measuring state is established. Through concrete analyses, the measure demands for getting a certain amount of a final entanglement are revealed. It is found that a maximally entangled final state can be obtained from any two given initial entangled states via swapping with a certain probability; however, a peculiar measure should be performed. Moreover, some distinct properties are revealed and analyzed. Such a study will be useful in quantum information processes.

  9. Spin-orbit influence on dz2-type surface state at Ta(110)

    NASA Astrophysics Data System (ADS)

    Wortelen, H.; Miyamoto, K.; Mirhosseini, H.; Okuda, T.; Kimura, A.; Thonig, D.; Henk, J.; Donath, M.

    2015-10-01

    The influence of spin-orbit interaction on an occupied surface state at Ta(110) is investigated with spin- and angle-resolved photoemission and electronic structure calculations. The surface state appears in a symmetry gap at a binding energy of 0.45 eV at Γ ¯ and exhibits a free-electron-like E (k∥) dispersion with an effective mass m*/me of about -1.35 along Γ ¯H ¯ . Photoemission results for excitation with s - and p -polarized light confirm the predicted dz2-type symmetry of the state close to Γ ¯. Spin-resolved data for finite k∥ reveal a pure Rashba-type spin texture with a Rashba parameter of 0.063 ±0.007 eV Å . These findings clearly prove a sizable impact of spin-orbit coupling on the dz2 surface state and resolve a longstanding disagreement on this issue.

  10. High spin states of [sup 84]Sr

    SciTech Connect

    Garcia Bermudez, G.; Baktash, C.; Abenante, V.; Griffin, H.C.; Halbert, M.L.; Hensley, D.C.; Johnson, N.R.; Lee, I.Y.; McGowan, F.K.; Riley, M.A.; Sarantites, D.G.; Semkow, T.M.; Stracener, D.W.; Virtanen, A. Joint Institute for Heavy-Ion Research, Oak Ridge, Tennessee 37831 Departamento de Fisica, Comision Nacional de Energia Atomica, 1429 Buenos Aires Department of Chemistry, Washington University, Saint Louis, Missouri 63130 Department of chemistry, University of Michigan, Ann Arbor, Michigan 48104 )

    1994-06-01

    High spin states of [sup 84]Sr nucleus excited through the [sup 52]Cr([sup 36]S,2[ital p]2[ital n]) reaction at 130 MeV energy were studied utilizing the Oak Ridge Compton-Suppression Spectrometer System. The level scheme has been extended up to probably [ital I][sup [pi

  11. Indistinguishability of pure orthogonal product states by LOCC

    NASA Astrophysics Data System (ADS)

    Zhang, Xiaoqian; Weng, Jian; Tan, Xiaoqing; Luo, Weiqi

    2017-07-01

    We construct two sets of incomplete and extendible quantum pure orthogonal product states (POPS) in general bipartite high-dimensional quantum systems, which are all indistinguishable by local operations and classical communication. The first set of POPS is composed of two parts which are C^m⊗ C^{n_1} with 5≤ m≤ n_1 and C^m⊗ C^{n_2} with 5≤ m ≤ n_2, where n_1 is odd and n_2 is even. The second one is in C^m⊗ C^n (m, n≥ 4). Some subsets of these two sets can be extended into complete sets that local indistinguishability can be decided by noncommutativity which quantifies the quantumness of a quantum ensemble. Our study shows quantum nonlocality without entanglement.

  12. Entanglement of three-qubit pure states in terms of teleportation capability

    SciTech Connect

    Lee, Soojoon; Joo, Jaewoo; Kim, Jaewan

    2005-08-15

    We define an entanglement measure, called the partial tangle, which represents the residual two-qubit entanglement of a three-qubit pure state. By its explicit calculations for three-qubit pure states, we show that the partial tangle is closely related to the faithfulness of a teleportation scheme over a three-qubit pure state.

  13. High-spin states in ^88Kr

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Lisetskiy, A. F.; Cizewski, J. A.; Krücken, R.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Becker, J. A.; Younes, W.

    2007-10-01

    High-spin states in ^88Kr have been studied following the fission of the ^226Th compound nucleus formed in a fusion-evaporation reaction (^18O at 91 MeV on ^208Pb). The Gammasphere array was used to detect γ-ray coincidences. High-spin states up to spin (14^+) and ˜8 MeV excitation energy have been established. The level scheme reported for ^88Kr in the spontaneous fission of ^248Cm [1] has been enriched and extended to higher spin and excitation energies. Differences between the level scheme reported in [1] and that obtained in the present work will be discussed. The observed experimental states are also compared with theoretical shell-model and interacting-boson-model-2 calculations. This work has been supported by the U.S. Department of Energy under Contracts No. DE-AC52-06NA25396 (LANL), W-7405-ENG-48 (LLNL) and AC03-76SF00098 (LBNL) and by the National Science Foundation (Rutgers). [1] T. Rzaca-Urban et al., Eur. Phys. J. A 9, 165 (2000).

  14. One-Qubit Reduced States of a Pure Many-Qubit State: Polygon Inequalities

    NASA Astrophysics Data System (ADS)

    Higuchi, A.; Sudbery, A.; Szulc, J.

    2003-03-01

    We show that a necessary and sufficient condition for a set of n one-qubit mixed states to be the reduced states of a pure n-qubit state is that their smaller eigenvalues should satisfy polygon inequalities: each of them must be no greater than the sum of the others.

  15. Surface bound states and spin currents in noncentrosymmetric superconductors.

    PubMed

    Vorontsov, A B; Vekhter, I; Eschrig, M

    2008-09-19

    We investigate the ground state properties of a noncentrosymmetric superconductor near a surface. We determine the spectrum of Andreev bound states due to surface-induced mixing of bands with opposite spin helicities for a Rashba-type spin-orbit coupling. We find that the order parameter suppression qualitatively changes the bound state spectrum. The spin structure of Andreev states leads to a spin supercurrent along the interface, which is strongly enhanced compared to the normal state spin current. Particle and hole coherence amplitudes show Faraday-like rotations of the spin along quasiparticle trajectories.

  16. Preserving coherent spin and squeezed spin states of a spin-1 Bose-Einstein condensate with rotary echoes

    NASA Astrophysics Data System (ADS)

    Zhang, Jun; Han, Yingying; Xu, Peng; Zhang, Wenxian

    2016-11-01

    A challenge in precision measurement with squeezed spin state arises from the spin dephasing due to stray magnetic fields. To suppress such environmental noises, we employ a continuous driving protocol, rotary echo, to enhance the spin coherence of a spin-1 Bose-Einstein condensate in stray magnetic fields. Our analytical and numerical results show that the coherent and the squeezed spin states are preserved for a significantly long time, compared to the free induction decay time, if the condition h τ =m π is met with h the pulse amplitude and τ pulse width. In particular, both the spin average and the spin squeezing, including the direction and the amplitude, are simultaneously fixed for a squeezed spin state. Our results point out a practical way to implement quantum measurements based on a spin-1 condensate beyond the standard quantum limit.

  17. Direct Measurement of the Flip-Flop Rate of Electron Spins in the Solid State

    NASA Astrophysics Data System (ADS)

    Dikarov, Ekaterina; Zgadzai, Oleg; Artzi, Yaron; Blank, Aharon

    2016-10-01

    Electron spins in solids have a central role in many current and future spin-based devices, ranging from sensitive sensors to quantum computers. Many of these apparatuses rely on the formation of well-defined spin structures (e.g., a 2D array) with controlled and well-characterized spin-spin interactions. While being essential for device operation, these interactions can also result in undesirable effects, such as decoherence. Arguably, the most important pure quantum interaction that causes decoherence is known as the "flip-flop" process, where two interacting spins interchange their quantum state. Currently, for electron spins, the rate of this process can only be estimated theoretically, or measured indirectly, under limiting assumptions and approximations, via spin-relaxation data. This work experimentally demonstrates how the flip-flop rate can be directly and accurately measured by examining spin-diffusion processes in the solid state for physically fixed spins. Under such terms, diffusion can occur only through this flip-flop-mediated quantum-state exchange and not via actual spatial motion. Our approach is implemented on two types of samples, phosphorus-doped 28Si and nitrogen vacancies in diamond, both of which are significantly relevant to quantum sensors and information processing. However, while the results for the former sample are conclusive and reveal a flip-flop rate of approximately 12.3 Hz, for the latter sample only an upper limit of approximately 0.2 Hz for this rate can be estimated.

  18. Spin transistor based on pure nonlocal Andreev reflection in EuO-graphene/superconductor/EuO-graphene nanostructure

    NASA Astrophysics Data System (ADS)

    Ang, Yee Sin; Ang, Lay Kee; Zhang, Chao; Ma, Zhongshui

    In graphene-magnetic-insulator hybrid structure such as graphene-Europium-oxide, proximity induced exchange interaction opens up a spin-dependent bandgap and spin splitting in the Dirac band. We show that such band topology allows pure crossed Andreev reflection to be generated exclusively without the parasitic local Andreev reflection and elastic cotunnelling over a wide range of bias and Fermi levels. We model the charge transport in an EuO-graphene/superconductor/EuO-graphene three-terminal device and found that the pure non-local conductance exhibits rapid on/off switching characteristic with a minimal subthreshold swing of ~ 20 mV. Non-local conductance oscillation is observed when the Fermi levels in the superconducting lead is varied. The oscillatory behavior is directly related to the quasiparticle propagation in the superconducting lead and hence can be used as a tool to probe the subgap quasiparticle mode in superconducting graphene. The non-local current is 100% spin-polarized and is highly tunable in our proposed device. This opens up the possibility of highly tunable graphene-based spin transistor that operates purely in the non-local transport regime.

  19. Geometric local invariants and pure three-qubit states

    SciTech Connect

    Williamson, Mark S.; Ericsson, Marie; Johansson, Markus; Sjoeqvist, Erik; Sudbery, Anthony; Vedral, Vlatko; Wootters, William K.

    2011-06-15

    We explore a geometric approach to generating local SU(2) and SL(2,C) invariants for a collection of qubits inspired by lattice gauge theory. Each local invariant or ''gauge'' invariant is associated with a distinct closed path (or plaquette) joining some or all of the qubits. In lattice gauge theory, the lattice points are the discrete space-time points, the transformations between the points of the lattice are defined by parallel transporters, and the gauge invariant observable associated with a particular closed path is given by the Wilson loop. In our approach the points of the lattice are qubits, the link transformations between the qubits are defined by the correlations between them, and the gauge invariant observable, the local invariants associated with a particular closed path, are also given by a Wilson looplike construction. The link transformations share many of the properties of parallel transporters, although they are not undone when one retraces one's steps through the lattice. This feature is used to generate many of the invariants. We consider a pure three-qubit state as a test case and find we can generate a complete set of algebraically independent local invariants in this way; however, the framework given here is applicable to generating local unitary invariants for mixed states composed of any number of d-level quantum systems. We give an operational interpretation of these invariants in terms of observables.

  20. Geometric local invariants and pure three-qubit states

    NASA Astrophysics Data System (ADS)

    Williamson, Mark S.; Ericsson, Marie; Johansson, Markus; Sjöqvist, Erik; Sudbery, Anthony; Vedral, Vlatko; Wootters, William K.

    2011-06-01

    We explore a geometric approach to generating local SU(2) and SL(2,C) invariants for a collection of qubits inspired by lattice gauge theory. Each local invariant or “gauge” invariant is associated with a distinct closed path (or plaquette) joining some or all of the qubits. In lattice gauge theory, the lattice points are the discrete space-time points, the transformations between the points of the lattice are defined by parallel transporters, and the gauge invariant observable associated with a particular closed path is given by the Wilson loop. In our approach the points of the lattice are qubits, the link transformations between the qubits are defined by the correlations between them, and the gauge invariant observable, the local invariants associated with a particular closed path, are also given by a Wilson looplike construction. The link transformations share many of the properties of parallel transporters, although they are not undone when one retraces one’s steps through the lattice. This feature is used to generate many of the invariants. We consider a pure three-qubit state as a test case and find we can generate a complete set of algebraically independent local invariants in this way; however, the framework given here is applicable to generating local unitary invariants for mixed states composed of any number of d-level quantum systems. We give an operational interpretation of these invariants in terms of observables.

  1. Optimal pulse spacing for dynamical decoupling in the presence of a purely dephasing spin bath

    NASA Astrophysics Data System (ADS)

    Ajoy, Ashok; Álvarez, Gonzalo A.; Suter, Dieter

    2011-03-01

    Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are C13 nuclear spins and the environment consists of a H1 nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.

  2. Optimal pulse spacing for dynamical decoupling in the presence of a purely dephasing spin bath

    SciTech Connect

    Ajoy, Ashok; Alvarez, Gonzalo A.; Suter, Dieter

    2011-03-15

    Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are {sup 13}C nuclear spins and the environment consists of a {sup 1}H nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.

  3. Spin-dependent quantum interference in photoemission process from spin-orbit coupled states.

    PubMed

    Yaji, Koichiro; Kuroda, Kenta; Toyohisa, Sogen; Harasawa, Ayumi; Ishida, Yukiaki; Watanabe, Shuntaro; Chen, Chuangtian; Kobayashi, Katsuyoshi; Komori, Fumio; Shin, Shik

    2017-02-24

    Spin-orbit interaction entangles the orbitals with the different spins. The spin-orbital-entangled states were discovered in surface states of topological insulators. However, the spin-orbital-entanglement is not specialized in the topological surface states. Here, we show the spin-orbital texture in a surface state of Bi(111) by laser-based spin- and angle-resolved photoelectron spectroscopy (laser-SARPES) and describe three-dimensional spin-rotation effect in photoemission resulting from spin-dependent quantum interference. Our model reveals that, in the spin-orbit-coupled systems, the spins pointing to the mutually opposite directions are independently locked to the orbital symmetries. Furthermore, direct detection of coherent spin phenomena by laser-SARPES enables us to clarify the phase of the dipole transition matrix element responsible for the spin direction in photoexcited states. These results permit the tuning of the spin polarization of optically excited electrons in solids with strong spin-orbit interaction.

  4. Spin-dependent quantum interference in photoemission process from spin-orbit coupled states

    NASA Astrophysics Data System (ADS)

    Yaji, Koichiro; Kuroda, Kenta; Toyohisa, Sogen; Harasawa, Ayumi; Ishida, Yukiaki; Watanabe, Shuntaro; Chen, Chuangtian; Kobayashi, Katsuyoshi; Komori, Fumio; Shin, Shik

    2017-02-01

    Spin-orbit interaction entangles the orbitals with the different spins. The spin-orbital-entangled states were discovered in surface states of topological insulators. However, the spin-orbital-entanglement is not specialized in the topological surface states. Here, we show the spin-orbital texture in a surface state of Bi(111) by laser-based spin- and angle-resolved photoelectron spectroscopy (laser-SARPES) and describe three-dimensional spin-rotation effect in photoemission resulting from spin-dependent quantum interference. Our model reveals that, in the spin-orbit-coupled systems, the spins pointing to the mutually opposite directions are independently locked to the orbital symmetries. Furthermore, direct detection of coherent spin phenomena by laser-SARPES enables us to clarify the phase of the dipole transition matrix element responsible for the spin direction in photoexcited states. These results permit the tuning of the spin polarization of optically excited electrons in solids with strong spin-orbit interaction.

  5. Strong Linear Dichroism in Spin-Polarized Photoemission from Spin-Orbit-Coupled Surface States.

    PubMed

    Bentmann, H; Maaß, H; Krasovskii, E E; Peixoto, T R F; Seibel, C; Leandersson, M; Balasubramanian, T; Reinert, F

    2017-09-08

    A comprehensive understanding of spin-polarized photoemission is crucial for accessing the electronic structure of spin-orbit coupled materials. Yet, the impact of the final state in the photoemission process on the photoelectron spin has been difficult to assess in these systems. We present experiments for the spin-orbit split states in a Bi-Ag surface alloy showing that the alteration of the final state with energy may cause a complete reversal of the photoelectron spin polarization. We explain the effect on the basis of ab initio one-step photoemission theory and describe how it originates from linear dichroism in the angular distribution of photoelectrons. Our analysis shows that the modulated photoelectron spin polarization reflects the intrinsic spin density of the surface state being sampled differently depending on the final state, and it indicates linear dichroism as a natural probe of spin-orbit coupling at surfaces.

  6. Strong Linear Dichroism in Spin-Polarized Photoemission from Spin-Orbit-Coupled Surface States

    NASA Astrophysics Data System (ADS)

    Bentmann, H.; Maaß, H.; Krasovskii, E. E.; Peixoto, T. R. F.; Seibel, C.; Leandersson, M.; Balasubramanian, T.; Reinert, F.

    2017-09-01

    A comprehensive understanding of spin-polarized photoemission is crucial for accessing the electronic structure of spin-orbit coupled materials. Yet, the impact of the final state in the photoemission process on the photoelectron spin has been difficult to assess in these systems. We present experiments for the spin-orbit split states in a Bi-Ag surface alloy showing that the alteration of the final state with energy may cause a complete reversal of the photoelectron spin polarization. We explain the effect on the basis of ab initio one-step photoemission theory and describe how it originates from linear dichroism in the angular distribution of photoelectrons. Our analysis shows that the modulated photoelectron spin polarization reflects the intrinsic spin density of the surface state being sampled differently depending on the final state, and it indicates linear dichroism as a natural probe of spin-orbit coupling at surfaces.

  7. ℬ(H) has a pure state that is not multiplicative on any masa

    PubMed Central

    Akemann, Charles; Weaver, Nik

    2008-01-01

    Assuming the continuum hypothesis, we prove that ℬ(H) has a pure state whose restriction to any masa is not pure. This resolves negatively old conjectures of Kadison and Singer and of Anderson. PMID:18378909

  8. B(H) has a pure state that is not multiplicative on any masa.

    PubMed

    Akemann, Charles; Weaver, Nik

    2008-04-08

    Assuming the continuum hypothesis, we prove that Bernoulli function(H) has a pure state whose restriction to any masa is not pure. This resolves negatively old conjectures of Kadison and Singer and of Anderson.

  9. Dressed photon-orbital states in a quantum dot: Intervalley spin resonance

    NASA Astrophysics Data System (ADS)

    Scarlino, P.; Kawakami, E.; Jullien, T.; Ward, D. R.; Savage, D. E.; Lagally, M. G.; Friesen, Mark; Coppersmith, S. N.; Eriksson, M. A.; Vandersypen, L. M. K.

    2017-04-01

    The valley degree of freedom is intrinsic to spin qubits in Si/SiGe quantum dots. It has been viewed alternately as a hazard, especially when the lowest valley-orbit splitting is small compared to the thermal energy, or as an asset, most prominently in proposals to use the valley degree of freedom itself as a qubit. Here we present experiments in which microwave electric field driving induces transitions between both valley-orbit and spin states. We show that this system is highly nonlinear and can be understood through the use of dressed photon-orbital states, enabling a unified understanding of the six microwave resonance lines we observe. Some of these resonances are intervalley spin transitions that arise from a nonadiabatic process in which both the valley and the spin degree of freedom are excited simultaneously. For these transitions, involving a change in valley-orbit state, we find a tenfold increase in sensitivity to electric fields and electrical noise compared to pure spin transitions, strongly reducing the phase coherence when changes in valley-orbit index are incurred. In contrast to this nonadiabatic transition, the pure spin transitions, whether arising from harmonic or subharmonic generation, are shown to be adiabatic in the orbital sector. The nonlinearity of the system is most strikingly manifest in the observation of a dynamical anticrossing between a spin-flip, intervalley transition and a three-photon transition enabled by the strong nonlinearity we find in this seemly simple system.

  10. Multiferroic behavior at a spin state transition

    NASA Astrophysics Data System (ADS)

    Zapf, Vivien; Chikara, Shalinee; Singleton, John; Lin, Shizeng; Batista, Cristian; Scott, Brian; Smythe, Nathan

    Traditionally, multiferroic behavior is studied in materials with coexisting long-range orders, such as ferromagnetism and ferroelectricity. Here we present multiferroic behavior at a spin-state transition (SST). SSTs, for example, the S = 1 to S = 2 transition in Mn3+ can become cooperative magneto-structural phase transitions due to structural coupling between ions. SSTs are accompanied by change in the orbital occupation and hence, strongly coupled to the lattice and charge degrees of freedom. They are a dominant functionality in metal-organic materials, persisting up to room temperature in some compounds. We demonstrate that a magnetic SST can induce ferroelectricity. We study a Mn-based metal-organic system in which a three-fold degenerate dynamic Jahn-Teller effect at high temperatures vanishes when the temperature is lowered, and the system drops into a lower spin state. Application of a magnetic field restores the high spin Jahn-Teller-active state and allows the Jahn Teller distortions to order cooperatively, creating a dielectric constant change and a net electric polarization. We use high magnetic fields at the NHMFL to study the magnetic and electric behavior of this system across a significant fraction of its T-H phase space, and compare to theoretical modeling.

  11. Spin susceptibility of Andreev bound states

    NASA Astrophysics Data System (ADS)

    Rosemeyer, B. M.; Vorontsov, Anton B.

    2016-10-01

    We calculate the electronic spin susceptibility and spin-lattice relaxation rate in a singlet superconductor near a pair-breaking surface, or in a domain wall of the order parameter. We directly link the presence of high-density Andreev bound states in the inhomogeneous region, combined with coherence factors, to the enhancement of the susceptibility above the normal state's value for certain q vectors. Besides the dominant peak at ferromagnetic vector q =0 , we find significant enhancement of antiferromagnetic correlations at vectors q ≲2 kf , with q along the domain wall in an S -wave superconductor, and across the domain wall in D -wave (nodes along the wall). These features are destroyed by applying a moderate Zeeman field that splits the zero-energy peak. We solve Bogoliubov-de Gennes equations in momentum space and discuss the deviation of our results from the lattice models investigated previously. Large enhancement of the spin-lattice relaxation rate T1-1 at the domain wall provides a clear signature of the quasiparticle bound states, and is in good agreement with recent experiment in organic superconductor κ -(BEDT-TTF ) 2Cu (NCS) 2 .

  12. Random pure states: Quantifying bipartite entanglement beyond the linear statistics

    NASA Astrophysics Data System (ADS)

    Vivo, Pierpaolo; Pato, Mauricio P.; Oshanin, Gleb

    2016-05-01

    We analyze the properties of entangled random pure states of a quantum system partitioned into two smaller subsystems of dimensions N and M . Framing the problem in terms of random matrices with a fixed-trace constraint, we establish, for arbitrary N ≤M , a general relation between the n -point densities and the cross moments of the eigenvalues of the reduced density matrix, i.e., the so-called Schmidt eigenvalues, and the analogous functionals of the eigenvalues of the Wishart-Laguerre ensemble of the random matrix theory. This allows us to derive explicit expressions for two-level densities, and also an exact expression for the variance of von Neumann entropy at finite N ,M . Then, we focus on the moments E {Ka} of the Schmidt number K , the reciprocal of the purity. This is a random variable supported on [1 ,N ] , which quantifies the number of degrees of freedom effectively contributing to the entanglement. We derive a wealth of analytical results for E {Ka} for N =2 and 3 and arbitrary M , and also for square N =M systems by spotting for the latter a connection with the probability P (xminGUE≥√{2 N }ξ ) that the smallest eigenvalue xminGUE of an N ×N matrix belonging to the Gaussian unitary ensemble is larger than √{2 N }ξ . As a by-product, we present an exact asymptotic expansion for P (xminGUE≥√{2 N }ξ ) for finite N as ξ →∞ . Our results are corroborated by numerical simulations whenever possible, with excellent agreement.

  13. Random pure states: Quantifying bipartite entanglement beyond the linear statistics.

    PubMed

    Vivo, Pierpaolo; Pato, Mauricio P; Oshanin, Gleb

    2016-05-01

    We analyze the properties of entangled random pure states of a quantum system partitioned into two smaller subsystems of dimensions N and M. Framing the problem in terms of random matrices with a fixed-trace constraint, we establish, for arbitrary N≤M, a general relation between the n-point densities and the cross moments of the eigenvalues of the reduced density matrix, i.e., the so-called Schmidt eigenvalues, and the analogous functionals of the eigenvalues of the Wishart-Laguerre ensemble of the random matrix theory. This allows us to derive explicit expressions for two-level densities, and also an exact expression for the variance of von Neumann entropy at finite N,M. Then, we focus on the moments E{K^{a}} of the Schmidt number K, the reciprocal of the purity. This is a random variable supported on [1,N], which quantifies the number of degrees of freedom effectively contributing to the entanglement. We derive a wealth of analytical results for E{K^{a}} for N=2 and 3 and arbitrary M, and also for square N=M systems by spotting for the latter a connection with the probability P(x_{min}^{GUE}≥sqrt[2N]ξ) that the smallest eigenvalue x_{min}^{GUE} of an N×N matrix belonging to the Gaussian unitary ensemble is larger than sqrt[2N]ξ. As a by-product, we present an exact asymptotic expansion for P(x_{min}^{GUE}≥sqrt[2N]ξ) for finite N as ξ→∞. Our results are corroborated by numerical simulations whenever possible, with excellent agreement.

  14. Computation of indirect nuclear spin-spin couplings with reduced complexity in pure and hybrid density functional approximations.

    PubMed

    Luenser, Arne; Kussmann, Jörg; Ochsenfeld, Christian

    2016-09-28

    We present a (sub)linear-scaling algorithm to determine indirect nuclear spin-spin coupling constants at the Hartree-Fock and Kohn-Sham density functional levels of theory. Employing efficient integral algorithms and sparse algebra routines, an overall (sub)linear scaling behavior can be obtained for systems with a non-vanishing HOMO-LUMO gap. Calculations on systems with over 1000 atoms and 20 000 basis functions illustrate the performance and accuracy of our reference implementation. Specifically, we demonstrate that linear algebra dominates the runtime of conventional algorithms for 10 000 basis functions and above. Attainable speedups of our method exceed 6 × in total runtime and 10 × in the linear algebra steps for the tested systems. Furthermore, a convergence study of spin-spin couplings of an aminopyrazole peptide upon inclusion of the water environment is presented: using the new method it is shown that large solvent spheres are necessary to converge spin-spin coupling values.

  15. Computation of indirect nuclear spin-spin couplings with reduced complexity in pure and hybrid density functional approximations

    NASA Astrophysics Data System (ADS)

    Luenser, Arne; Kussmann, Jörg; Ochsenfeld, Christian

    2016-09-01

    We present a (sub)linear-scaling algorithm to determine indirect nuclear spin-spin coupling constants at the Hartree-Fock and Kohn-Sham density functional levels of theory. Employing efficient integral algorithms and sparse algebra routines, an overall (sub)linear scaling behavior can be obtained for systems with a non-vanishing HOMO-LUMO gap. Calculations on systems with over 1000 atoms and 20 000 basis functions illustrate the performance and accuracy of our reference implementation. Specifically, we demonstrate that linear algebra dominates the runtime of conventional algorithms for 10 000 basis functions and above. Attainable speedups of our method exceed 6 × in total runtime and 10 × in the linear algebra steps for the tested systems. Furthermore, a convergence study of spin-spin couplings of an aminopyrazole peptide upon inclusion of the water environment is presented: using the new method it is shown that large solvent spheres are necessary to converge spin-spin coupling values.

  16. Canonical form of three-fermion pure-states with six single particle states

    SciTech Connect

    Chen, Lin; Ž Ðoković, Dragomir; Grassl, Markus; Zeng, Bei

    2014-08-01

    We construct a canonical form for pure states in Λ³(C⁶), the three-fermion system with six single particle states, under local unitary (LU) transformations, i.e., the unitary group U(6). We also construct a minimal set of generators of the algebra of polynomial U(6)-invariants on Λ³(C⁶). It turns out that this algebra is isomorphic to the algebra of polynomial LU-invariants of three-qubits which are additionally invariant under qubit permutations. As a consequence of this surprising fact, we deduce that there is a one-to-one correspondence between the U(6)-orbits of pure three-fermion states in Λ³(C⁶) and the LU orbits of pure three-qubit states when qubit permutations are allowed. As an important byproduct, we obtain a new canonical form for pure three-qubit states under LU transformations U(2) × U(2) × U(2) (no qubit permutations allowed)

  17. Correlations and Werner states in finite spin linear arrays

    NASA Astrophysics Data System (ADS)

    Wells, P. R.; Chaves, C. M.; d'Albuquerque e Castro, J.; Koiller, Belita

    2013-10-01

    Pairwise quantum correlations in the ground state of an N-spins antiferromagnetic Heisenberg chain are investigated. By varying the exchange coupling between two neighboring sites, it is possible to reversibly drive spins from entangled to disentangled states. For even N, the two-spin density matrix is written in the form of a Werner state, allowing identification of its single parameter with the usual spin-spin correlation function. The N = 4 chain is identified as a promising system for practical demonstrations of non-classical correlations and the realization of Werner states in familiar condensed matter systems. Fabrication and measurement ingredients are within current capabilities.

  18. The tumbling spin state of (99942) Apophis

    NASA Astrophysics Data System (ADS)

    Pravec, P.; Scheirich, P.; Ďurech, J.; Pollock, J.; Kušnirák, P.; Hornoch, K.; Galád, A.; Vokrouhlický, D.; Harris, A. W.; Jehin, E.; Manfroid, J.; Opitom, C.; Gillon, M.; Colas, F.; Oey, J.; Vraštil, J.; Reichart, D.; Ivarsen, K.; Haislip, J.; LaCluyze, A.

    2014-05-01

    Our photometric observations of Asteroid (99942) Apophis from December 2012 to April 2013 revealed it to be in a state of non-principal axis rotation (tumbling). We constructed its spin and shape model and found that it is in a moderately excited Short Axis Mode (SAM) state with a ratio of the rotational kinetic energy to the basic spin state energy E/E0=1.024±0.013. (All quoted uncertainties correspond to 3σ.) The greatest and intermediate principal moments of inertia are nearly the same with I2/I3=0.965-0.015+0.009, but the smallest principal moment of inertia is substantially lower with I1/I3=0.61-0.08+0.11; the asteroid’s dynamically equivalent ellipsoid is close to a prolate ellipsoid. The precession and rotation periods are Pϕ=27.38±0.07 h and Pψ=263±6 h, respectively; the strongest observed lightcurve amplitude for the SAM case is in the 2nd harmonic of P1=P=30.56±0.01 h. The rotation is retrograde with the angular momentum vector’s ecliptic longitude and latitude of 250° and -75° (the uncertainty area is approximately an ellipse with the major and minor semiaxes of 27° and 14°, respectively). An implication of the retrograde rotation is a somewhat increased probability of the Apophis’ impact in 2068, but it is still very small with the risk level on the Palermo Scale remaining well below zero. Apophis is a member of the population of slowly tumbling asteroids. Applying the theory of asteroid nutational damping by Breiter et al. (Breiter, S., Rożek, A., Vokrouhlický, D. [2012]. Mon. Not. R. Astron. Soc. 427, 755-769), we found that slowly tumbling asteroids predominate in the spin rate-size range where their estimated damping times are greater than about 0.2 Gyr. The appearance that the PA/NPA rotators transition line seems to follow a line of constant damping time may be because there are two or more asteroid spin evolution mechanisms in play, or the factor of μQ (the elastic modulus times the quality factor) is not constant but it may

  19. Bidirectional teleportation of a pure EPR state by using GHZ states

    NASA Astrophysics Data System (ADS)

    Hassanpour, Shima; Houshmand, Monireh

    2016-02-01

    In the present paper, a novel bidirectional quantum teleportation protocol is proposed. By using entanglement swapping technique, two GHZ states are shared as a quantum channel between Alice and Bob as legitimate users. In this scheme, based on controlled-not operation, single-qubit measurement, and appropriate unitary operations, two users can simultaneously transmit a pure EPR state to each other, While, in the previous protocols, the users can just teleport a single-qubit state to each other via more than four-qubit state. Therefore, the proposed scheme is economical compared with previous protocols.

  20. Generation of pure spin currents via Auger recombination in quantum wells with Rashba splitting

    SciTech Connect

    Afanasiev, A. N. Greshnov, A. A. Greshnov, A. A.

    2015-10-15

    We propose a nonoptical mechanism for generating spin current via Auger recombination in semiconductor quantum wells (QWs) with spin–orbit splitting associated with structural QW asymmetry. It is shown that Auger recombination in narrow-bandgap semiconductors makes it possible to produce spin currents that exceed those that are obtained in the case of intraband as well as interband optical excitation. Analysis shows that the interference term in the expression for the Auger-recombination rate is responsible for the generation of spin currents.

  1. Quantum logical operations for spin 3/2 quadrupolar nuclei monitored by quantum state tomography.

    PubMed

    Bonk, F A; deAzevedo, E R; Sarthour, R S; Bulnes, J D; Freitas, J C C; Guimarães, A P; Oliveira, I S; Bonagamba, T J

    2005-08-01

    This article presents the realization of many self-reversible quantum logic gates using two-qubit quadrupolar spin 3/2 systems. Such operations are theoretically described using propagation matrices for the RF pulses that include the effect of the quadrupolar evolution during the pulses. Experimental demonstrations are performed using a generalized form of the recently developed method for quantum state tomography in spin 3/2 systems. By doing so, the possibility of controlling relative phases of superimposed pseudo-pure states is demonstrated. In addition, many aspects of the effect of the quadrupolar evolution, occurring during the RF pulses, on the quantum operations performance are discussed. Most of the procedures presented can be easily adapted to describe selective pulses of higher spin systems (>3/2) and for spin 1/2 under J couplings.

  2. Coexistence of pure and mixed states in nonlinear maps

    NASA Astrophysics Data System (ADS)

    Roth, Yehuda

    2015-09-01

    Coherence and interaction are important concepts in physics. While interaction describes a relation between individual objects such as forces acting between distinguishable particles, coherent objects exist with the sole purpose of describing a single object. For example, each component of a vector provides us with only partial information. The whole picture is revealed only when the components are coherently related to their generating vector. Another example is a singlet of two spin ½- particles. The true nature of these two coherent particles is described by a spin-less single particle. Apparently it seems that objects can be either coherent or lion-coherent but they cannot be both simultaneously. This is almost true. We show that a system can be described simultaneously as coherent and lion-coherent but an observer can distinguish only one concept at a time.

  3. Single-Shot Ternary Readout of Two-Electron Spin States in a Quantum Dot Using Spin Filtering by Quantum Hall Edge States.

    PubMed

    Kiyama, H; Nakajima, T; Teraoka, S; Oiwa, A; Tarucha, S

    2016-12-02

    We report on the single-shot readout of three two-electron spin states-a singlet and two triplet substates-whose z components of spin angular momentum are 0 and +1, in a gate-defined GaAs single quantum dot. The three spin states are distinguished by detecting spin-dependent tunnel rates that arise from two mechanisms: spin filtering by spin-resolved edge states and spin-orbital correlation with orbital-dependent tunneling. The three states form one ground state and two excited states, and we observe the spin relaxation dynamics among the three spin states.

  4. Symmetry rules shaping spin-orbital textures in surface states

    NASA Astrophysics Data System (ADS)

    Gotlieb, Kenneth; Li, Zhenglu; Lin, Chiu-Yun; Jozwiak, Chris; Ryoo, Ji Hoon; Park, Cheol-Hwan; Hussain, Zahid; Louie, Steven G.; Lanzara, Alessandra

    2017-06-01

    Strong spin-orbit coupling creates exotic electronic states such as Rashba and topological surface states, which hold promise for technologies involving the manipulation of spin. Only recently has the complexity of these surface states been appreciated: they are composed of several atomic orbitals with distinct spin textures in momentum space. A complete picture of the wave function must account for this orbital dependence of spin. We discover that symmetry constrains the way orbital and spin components of a state coevolve as a function of momentum, and from this, we determine the rules governing how the two degrees of freedom are interwoven. We directly observe this complexity in spin-resolved photoemission and ab initio calculations of the topological surface states of Sb(111), where the photoelectron spin direction near Γ ¯ is found to have a strong and unusual dependence on photon polarization. This dependence unexpectedly breaks down at large |k | , where the surface states mix with other nearby surface states. However, along mirror planes, symmetry protects the distinct spin orientations of different orbitals. Our discovery broadens the understanding of surface states with strong spin-orbit coupling, demonstrates the conditions that allow for optical manipulation of photoelectron spin, and will be highly instructive for future spintronics applications.

  5. High-spin states in 208Rn

    NASA Astrophysics Data System (ADS)

    Triggs, W. J.; Poletti, A. R.; Dracoulis, G. D.; Fahlander, C.; Byrne, A. P.

    1983-03-01

    The yrast decay scheme of 208Rn has been investigated up to spin ≈ 20 h̵ and an excitation energy of ≈ 6 MeV. Several different γ-ray spectroscopic techniques were used to determine the properties of excited states and transitions in the nucleus. Significant changes to the previously established level scheme are proposed, based on the existence of an unobserved 3.1 keV transition. Simple empirical shell-model calculations of level energies aided in the assignment of shell-model configurations to excited states and the decay scheme is discussed in terms of these configurations. The energy level systematics for the even radon isotopes, from A = 206 to 212 are discussed, as are core polarization effects in the even radon isotopes ( A = 204 to 210) and polonium isotopes ( A = 202-208).

  6. Magnetic field sensors using 13-spin cat states

    SciTech Connect

    Simmons, Stephanie; Karlen, Steven D.; Jones, Jonathan A.; Ardavan, Arzhang; Morton, John J. L.

    2010-08-15

    Measurement devices could benefit from entangled correlations to yield a measurement sensitivity approaching the physical Heisenberg limit. Building upon previous magnetometric work using pseudoentangled spin states in solution-state NMR, we present two conceptual advancements to better prepare and interpret the pseudoentanglement resource. We apply these to a 13-spin cat state to measure the local magnetic field with a 12.2 sensitivity increase over an equivalent number of isolated spins.

  7. From local to global ground states in Ising spin glasses

    NASA Astrophysics Data System (ADS)

    Zintchenko, Ilia; Hastings, Matthew B.; Troyer, Matthias

    2015-01-01

    We consider whether it is possible to find ground states of frustrated spin systems by solving them locally. Using spin glass physics and Imry-Ma arguments in addition to numerical benchmarks we quantify the power of such local solution methods and show that for the average low-dimensional spin glass problem outside the spin glass phase the exact ground state can be found in polynomial time. In the second part we present a heuristic, general-purpose hierarchical approach which for spin glasses on chimera graphs and lattices in two and three dimensions outperforms, to our knowledge, any other solver currently around, with significantly better scaling performance than simulated annealing.

  8. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES: On Superconductivity State in Pure Graphene

    NASA Astrophysics Data System (ADS)

    Mousavi, Hamze

    2010-10-01

    We study theoretically the possibility of superconductivity state in pure graphene within the extended attractive Hubbard model. In the absence of disorder, when we use the local attractive interaction potential, U ⋍ 5t, where t is hopping term, pure graphene can be in superconductivity state.

  9. Universally coupled massive gravity, III: dRGT-Maheshwari pure spin-2, Ogievetsky-Polubarinov and arbitrary mass terms

    NASA Astrophysics Data System (ADS)

    Pitts, J. Brian

    2016-02-01

    Einstein's equations were derived for a free massless spin-2 field using universal coupling in the 1950-1970s by various authors; total stress-energy including gravity's served as a source for linear free field equations. A massive variant was likewise derived in the late 1960s by Freund, Maheshwari and Schonberg, and thought to be unique. How broad is universal coupling? In the last decade four 1-parameter families of massive spin-2 theories (contravariant, covariant, tetrad, and cotetrad of almost any density weights) have been derived using universal coupling. The (co)tetrad derivations included 2 of the 3 pure spin-2 theories due to de Rham, Gabadadze, and Tolley; those two theories first appeared in the 2-parameter Ogievetsky-Polubarinov family (1965), which developed the symmetric square root of the metric as a nonlinear group realization. One of the two theories was identified as pure spin-2 by Maheshwari in 1971-1972, thus evading the Boulware-Deser-Tyutin-Fradkin ghost by the time it was announced. Unlike the previous 4 families, this paper permits nonlinear field redefinitions to build the effective metric. By not insisting in advance on knowing the observable significance of the graviton potential to all orders, one finds that an arbitrary graviton mass term can be derived using universal coupling. The arbitrariness of a universally coupled mass/self-interaction term contrasts sharply with the uniqueness of the Einstein kinetic term. One might have hoped to use universal coupling as a tie-breaking criterion for choosing among theories that are equally satisfactory on more crucial grounds (such as lacking ghosts and having a smooth massless limit). But the ubiquity of universal coupling implies that the criterion does not favor any particular theories among those with the Einstein kinetic term.

  10. Universally coupled massive gravity, III: dRGT–Maheshwari pure spin-2, Ogievetsky–Polubarinov and arbitrary mass terms

    SciTech Connect

    Pitts, J. Brian

    2016-02-15

    Einstein’s equations were derived for a free massless spin-2 field using universal coupling in the 1950–1970s by various authors; total stress–energy including gravity’s served as a source for linear free field equations. A massive variant was likewise derived in the late 1960s by Freund, Maheshwari and Schonberg, and thought to be unique. How broad is universal coupling? In the last decade four 1-parameter families of massive spin-2 theories (contravariant, covariant, tetrad, and cotetrad of almost any density weights) have been derived using universal coupling. The (co)tetrad derivations included 2 of the 3 pure spin-2 theories due to de Rham, Gabadadze, and Tolley; those two theories first appeared in the 2-parameter Ogievetsky–Polubarinov family (1965), which developed the symmetric square root of the metric as a nonlinear group realization. One of the two theories was identified as pure spin-2 by Maheshwari in 1971–1972, thus evading the Boulware–Deser–Tyutin–Fradkin ghost by the time it was announced. Unlike the previous 4 families, this paper permits nonlinear field redefinitions to build the effective metric. By not insisting in advance on knowing the observable significance of the graviton potential to all orders, one finds that an arbitrary graviton mass term can be derived using universal coupling. The arbitrariness of a universally coupled mass/self-interaction term contrasts sharply with the uniqueness of the Einstein kinetic term. One might have hoped to use universal coupling as a tie-breaking criterion for choosing among theories that are equally satisfactory on more crucial grounds (such as lacking ghosts and having a smooth massless limit). But the ubiquity of universal coupling implies that the criterion does not favor any particular theories among those with the Einstein kinetic term.

  11. Optical Polarization Möbius Strips and Points of Purely Transverse Spin Density.

    PubMed

    Bauer, Thomas; Neugebauer, Martin; Leuchs, Gerd; Banzer, Peter

    2016-07-01

    Tightly focused light beams can exhibit complex and versatile structured electric field distributions. The local field may spin around any axis including a transverse axis perpendicular to the beams' propagation direction. At certain focal positions, the corresponding local polarization ellipse can even degenerate into a perfect circle, representing a point of circular polarization or C point. We consider the most fundamental case of a linearly polarized Gaussian beam, where-upon tight focusing-those C points created by transversely spinning fields can form the center of 3D optical polarization topologies when choosing the plane of observation appropriately. Because of the high symmetry of the focal field, these polarization topologies exhibit nontrivial structures similar to Möbius strips. We use a direct physical measure to find C points with an arbitrarily oriented spinning axis of the electric field and experimentally investigate the fully three-dimensional polarization topologies surrounding these C points by exploiting an amplitude and phase reconstruction technique.

  12. High spin states in 78Sr

    NASA Astrophysics Data System (ADS)

    Gross, C. J.; Heese, J.; Lieb, K. P.; Lister, C. J.; Varley, B. J.; Chishti, A. A.; McNeill, J. H.; Gelletly, W.

    1989-05-01

    78Sr was produced in the reaction 58Ni(24Mg, 2p2n) with a relative cross section of less than 2.5% of the total fusion cross section at 110 MeV, but high spin states up to 16ħ were firmly identified. Fifteen neutron detectors and fifteen Compton suppressed Ge detectors were used in a large solid angle arrangement. 2nγγ and nγγ coincidences were recorded. A small irregularity in the dynamic moment of inertia J(2)/ħ2 is evidence for a strongly mixed band crossing at ħω~=0.55 MeV in agreement with what is observed in 80,82Sr.

  13. Concurrence of assistance and Mermin inequality on three-qubit pure states

    SciTech Connect

    Chi, Dong Pyo; Kim, Taewan; Lee, Kyungjin; Jeong, Kabgyun; Lee, Soojoon

    2010-04-15

    We study a relation between the concurrence of assistance and the Mermin inequality on three-qubit pure states and claim that if a three-qubit pure state has a minimal concurrence of assistance greater than 1/2 then the state violates some Mermin inequality. In this work, we analytically show that our claim holds for several classes and also find that it can be generalized to the set of all three-qubit pure states by exploiting previous numerical work [C. Emary and C. W. J. Beenakker, Phys. Rev. A 69, 032317 (2004)].

  14. Rashba Spin-Orbit Coupling in Image Potential States

    NASA Astrophysics Data System (ADS)

    Tognolini, S.; Achilli, S.; Longetti, L.; Fava, E.; Mariani, C.; Trioni, M. I.; Pagliara, S.

    2015-07-01

    The search in two-dimensional condensed matter systems of Rashba-type spin-polarized electronic states is aimed by the possibility to control and manipulate the spin orientation. In this Letter, for the first time, we report on the experimental evidence of a Rashba-type spin splitting in the n =1 image potential state. The image potential state Rashba splitting here measured at the graphene/Ir(111) interface, as confirmed by theoretical considerations, can be detectable to any metal surface with a significant spin-orbit coupling.

  15. Robust state transfer in the quantum spin channel via weak measurement and quantum measurement reversal

    NASA Astrophysics Data System (ADS)

    He, Zhi; Yao, Chunmei; Zou, Jian

    2013-10-01

    Using the weak measurement (WM) and quantum measurement reversal (QMR) approach, robust state transfer and entanglement distribution can be realized in the spin-(1)/(2) Heisenberg chain. We find that the ultrahigh fidelity and long distance of quantum state transfer with certain success probability can be obtained using proper WM and QMR, i.e., the average fidelity of a general pure state from 80% to almost 100%, which is almost size independent. We also find that the distance and quality of entanglement distribution for the Bell state and the general Werner mixed state can be obviously improved by the WM and QMR approach.

  16. Generating Entangled Spin States for Quantum Metrology by Single-Photon Detection

    NASA Astrophysics Data System (ADS)

    McConnell, Robert; Zhang, Hao; Cuk, Senka; Hu, Jiazhong; Schleier-Smith, Monika; Vuletic, Vladan

    2014-05-01

    We present a proposal and latest experimental results on a probabilistic but heralded scheme to generate non-Gaussian entangled states of collective spin in large atomic ensembles by means of single-photon detection. One photon announces the preparation of a Dicke state, while two or more photons announce Schrödinger cat states. The entangled states thus produced allow interferometry below the Standard Quantum Limit (SQL). The method produces nearly pure states even for finite photon detection efficiency and weak atom-photon coupling. The entanglement generation can be made quasi-deterministic by means of repeated trial and feedback.

  17. High-spin states in 127I

    NASA Astrophysics Data System (ADS)

    Ding, B.; Zhang, Y. H.; Zhou, X. H.; Dong, G. X.; Xu, F. R.; Liu, M. L.; Li, G. S.; Zhang, N. T.; Wang, H. X.; Zhou, H. B.; Ma, Y. J.; Sasakiz, Y.; Yamada, K.; Ohshima, H.; Yokose, S.; Ishizuka, M.; Komatsubara, T.; Furuno, K.

    2012-04-01

    In-beam γ spectroscopy of the stable nucleus 127I has been studied experimentally using the 124Sn(7Li, 4nγ)127I reaction at a beam energy of 32 MeV. The high-spin level scheme of 127I is extended significantly. Negative-parity levels built on the 11/2-, πh11/2 particle state are observed up to (35/2-) and described as a decoupled band, extending our knowledge of decoupled structures to the most neutron-rich stable iodine isotope. Two ΔI=2 yrast positive-parity sequences are proposed to be associated with the πg7/2 configuration due to observations of several strong interband transitions, and two weakly populated ΔI=2 positive-parity bands are newly identified and interpreted as arising mainly from the πd5/2 configuration. Three-quasiparticle configurations are assigned to the Iπ=15/2+ and 23/2+ states according to the existing knowledge in neighboring nuclei; irregular noncollective and regular collective excitations built on these two (15/2+ and 23/2+) states are observed to coexist at similar energies. The observed three-quasiparticle band structures are further interpreted with the aid of configuration-constrained potential energy surface calculations.

  18. Atom lasers, coherent states, and coherence. I. Physically realizable ensembles of pure states

    NASA Astrophysics Data System (ADS)

    Wiseman, H. M.; Vaccaro, John A.

    2002-04-01

    A laser, be it an optical laser or an atom laser, is an open quantum system that produces a coherent beam of bosons (photons or atoms, respectively). Far above threshold, the stationary state ρss of the laser mode is a mixture of coherent-field states with random phase, or, equivalently, a Poissonian mixture of number states. This paper answers the question: can descriptions such as these, of ρss as a stationary ensemble of pure states, be physically realized? Here physical realization is as defined previously by us [H. M. Wiseman and J. A. Vaccaro, Phys. Lett. A 250, 241 (1998)]: an ensemble of pure states for a particular system can be physically realized if, without changing the dynamics of the system, an experimenter can (in principle) know at any time that the system is in one of the pure-state members of the ensemble. Such knowledge can be obtained by monitoring the baths to which the system is coupled, provided that coupling is describable by a Markovian master equation. Using a family of master equations for the (atom) laser, we solve for the physically realizable (PR) ensembles. We find that for any finite self-energy χ of the bosons in the laser mode, the coherent-state ensemble is not PR; the closest one can come to it is an ensemble of squeezed states. This is particularly relevant for atom lasers, where the self-energy arising from elastic collisions is expected to be large. By contrast, the number-state ensemble is always PR. As the self-energy χ increases, the states in the PR ensemble closest to the coherent-state ensemble become increasingly squeezed. Nevertheless, there are values of χ for which states with well-defined coherent amplitudes are PR, even though the atom laser is not coherent (in the sense of having a Bose-degenerate output). We discuss the physical significance of this anomaly in terms of conditional coherence (and hence conditional Bose degeneracy).

  19. Generalized concurrence measure for faithful quantification of multiparticle pure state entanglement using Lagrange's identity and wedge product

    NASA Astrophysics Data System (ADS)

    Bhaskara, Vineeth S.; Panigrahi, Prasanta K.

    2017-05-01

    Concurrence, introduced by Hill and Wootters (Phys Rev Lett 78:5022, 1997), provides an important measure of entanglement for a general pair of qubits that is faithful: strictly positive for entangled states and vanishing for all separable states. Such a measure captures the entire content of entanglement, providing necessary and sufficient conditions for separability. We present an extension of concurrence to multiparticle pure states in arbitrary dimensions by a new framework using the Lagrange's identity and wedge product representation of separability conditions, which coincides with the "I-concurrence" of Rungta et al. (Phys Rev A 64:042315, 2001) who proposed by extending Wootters's spin-flip operator to a so-called universal inverter superoperator. Our framework exposes an inherent geometry of entanglement and may be useful for the further extensions to mixed and continuous variable states.

  20. Spectroscopy of composite solid-state spin environments in diamond

    NASA Astrophysics Data System (ADS)

    Bar-Gill, Nir; Linh Pham, My; Belthangady, Chinmay; Le Sage, David; Lukin, Mikhail; Yacoby, Amir; Cappellaro, Paola; Walsworth, Ronald

    2012-06-01

    We apply dynamical decoupling pulse sequences to nitrogen-vacancy centers in diamond in order to spectrally decompose the dynamics of their spin environment, which consists of nuclear and electronic spin impurities. We study a variety of diamond samples to identify the dynamics of the different spin baths and the interplay between them. These results are useful for the basic understanding of spin dynamics in solid-state systems and the central spin problem and could inform efforts in engineering optimized samples for collective quantum information processing and quantum metrology.

  1. High-spin states in the 94Nb nucleus

    NASA Astrophysics Data System (ADS)

    Mărginean, N.; Bucurescu, D.; Căta-Danil, Ghe.; Căta-Danil, I.; Ivaşcu, M.; Ur, C. A.

    2000-09-01

    High-spin states have been studied for the first time in the 94Nb nucleus with the reaction 82Se(19F,α3nγ) at 68 MeV. A cascade of transitions has been observed, based on the (6)+ ground state and extending up to 6.5 MeV excitation and spin of about 19.

  2. Unidirectional electric field-induced spin-state switching in spin crossover based microelectronic devices

    NASA Astrophysics Data System (ADS)

    Lefter, Constantin; Tan, Reasmey; Dugay, Julien; Tricard, Simon; Molnár, Gábor; Salmon, Lionel; Carrey, Julian; Nicolazzi, William; Rotaru, Aurelian; Bousseksou, Azzedine

    2016-01-01

    We report on a molecular spin-state switching phenomenon induced by an electric field in micrometric objects of the [Fe(Htrz)2(trz)](BF4) spin crossover complex, organized between interdigitated electrodes. By applying an electric field step of 40 kV/cm at temperatures within the thermal hysteresis region of the first-order spin transition, the iron(II) ions are switched from the metastable high spin to the stable low spin state obtaining a rather incomplete transition but perfectly reversible by heating. A model based on the interaction between the electric field and the electric dipolar moment of spin crossover complexes, grasps the main features of the experimental data.

  3. Pure-state dynamics of a pair of charge qubits in a random environment

    NASA Astrophysics Data System (ADS)

    Burić, Nikola

    2005-10-01

    A pair of charge qubits in a random electromagnetic environment is studied, using the description of the random dynamics of its pure-state vector as given by quantum-state diffusion theory. It is shown by numerical computations that the pure-state dynamics provides a more detailed description than the density-matrix picture of the main effects such as phase dumping and depolarization.

  4. Pure Gaussian states from quantum harmonic oscillator chains with a single local dissipative process

    NASA Astrophysics Data System (ADS)

    Ma, Shan; Woolley, Matthew J.; Petersen, Ian R.; Yamamoto, Naoki

    2017-03-01

    We study the preparation of entangled pure Gaussian states via reservoir engineering. In particular, we consider a chain consisting of (2\\aleph +1) quantum harmonic oscillators where the central oscillator of the chain is coupled to a single reservoir. We then completely parametrize the class of (2\\aleph +1) -mode pure Gaussian states that can be prepared by this type of quantum harmonic oscillator chain. This parametrization allows us to determine the steady-state entanglement properties of such quantum harmonic oscillator chains.

  5. Pure-state dynamics of a pair of charge qubits in a random environment

    SciTech Connect

    Buric, Nikola

    2005-10-15

    A pair of charge qubits in a random electromagnetic environment is studied, using the description of the random dynamics of its pure-state vector as given by quantum-state diffusion theory. It is shown by numerical computations that the pure-state dynamics provides a more detailed description than the density-matrix picture of the main effects such as phase dumping and depolarization.

  6. Putting a new spin on unoccupied electronic states

    NASA Astrophysics Data System (ADS)

    Donath, Markus

    2015-03-01

    Inverse photoemission provides experimental information on the unoccupied electronic states, which is complementary to that obtained by photoemission about the occupied states. The first experimental demonstration of inverse photoemission in the vacuum ultraviolet energy range in 1977 was followed by an important add-on in 1982, the use of spin-polarized electrons. This pioneering experiment opened the way to reveal the spin character of unoccupied electron states in ferromagnets. In this contribution, I will describe the technical development of spin-resolved inverse photoemission with respect to efficiency as well as energy, momentum and spin resolution since the beginning until today. I will give a review about important results obtained by this technique. For about three decades, exchange-split electron states of majority and minority spin character at ferromagnetic surfaces and in ultrathin films were the topics of interest. Since recently, spin textures in momentum space caused by spin-orbit interaction in Rashba systems and topological insulators offer a new field of application for spin-resolved inverse photoemission. I will present a selection of examples, from small and giant Rashba splittings to rotating spins with chiral texture, influenced by the specific symmetry of the system and the orbital character of the respective states.

  7. Entanglement and extreme spin squeezing of unpolarized states

    NASA Astrophysics Data System (ADS)

    Vitagliano, Giuseppe; Apellaniz, Iagoba; Kleinmann, Matthias; Lücke, Bernd; Klempt, Carsten; Tóth, Géza

    2017-01-01

    We present criteria to detect the depth of entanglement in macroscopic ensembles of spin-j particles using the variance and second moments of the collective spin components. The class of states detected goes beyond traditional spin-squeezed states by including Dicke states and other unpolarized states. The criteria derived are easy to evaluate numerically even for systems of very many particles and outperform past approaches, especially in practical situations where noise is present. We also derive analytic lower bounds based on the linearization of our criteria, which make it possible to define spin-squeezing parameters for Dicke states. In addition, we obtain spin squeezing parameters also from the condition derived in (Sørensen and Mølmer 2001 Phys. Rev. Lett. 86 4431). We also extend our results to systems with fluctuating number of particles.

  8. Incommensurate antiferromagnetism in a pure spin system via cooperative organization of local and itinerant moments

    PubMed Central

    Feng, Yejun; Wang, Jiyang; Silevitch, D. M.; Mihaila, B.; Kim, J. W.; Yan, J.-Q.; Schulze, R. K.; Woo, Nayoon; Palmer, A.; Ren, Y.; van Wezel, Jasper; Littlewood, P. B.; Rosenbaum, T. F.

    2013-01-01

    Materials with strong correlations are prone to spin and charge instabilities, driven by Coulomb, magnetic, and lattice interactions. In materials that have significant localized and itinerant spins, it is not obvious which will induce order. We combine electrical transport, X-ray magnetic diffraction, and photoemission studies with band structure calculations to characterize successive antiferromagnetic transitions in GdSi. GdSi has both sizable local moments and a partially nested Fermi surface, without confounding contributions from orbital effects. We identify a route to incommensurate order where neither type of moment dominates, but is rooted in cooperative feedback between them. The nested Fermi surface of the itinerant electrons induces strong interactions between local moments at the nesting vector, whereas the ordered local moments in turn provide the necessary coupling for a spin-density wave to form among the itinerant electrons. This mechanism echoes the cooperative interactions between electrons and ions in charge-density–wave materials, and should be germane across a spectrum of transition-metal and rare-earth intermetallic compounds. PMID:23401555

  9. Spin-dependent quantum interference in photoemission process from spin-orbit coupled states

    PubMed Central

    Yaji, Koichiro; Kuroda, Kenta; Toyohisa, Sogen; Harasawa, Ayumi; Ishida, Yukiaki; Watanabe, Shuntaro; Chen, Chuangtian; Kobayashi, Katsuyoshi; Komori, Fumio; Shin, Shik

    2017-01-01

    Spin–orbit interaction entangles the orbitals with the different spins. The spin–orbital-entangled states were discovered in surface states of topological insulators. However, the spin–orbital-entanglement is not specialized in the topological surface states. Here, we show the spin–orbital texture in a surface state of Bi(111) by laser-based spin- and angle-resolved photoelectron spectroscopy (laser-SARPES) and describe three-dimensional spin-rotation effect in photoemission resulting from spin-dependent quantum interference. Our model reveals that, in the spin–orbit-coupled systems, the spins pointing to the mutually opposite directions are independently locked to the orbital symmetries. Furthermore, direct detection of coherent spin phenomena by laser-SARPES enables us to clarify the phase of the dipole transition matrix element responsible for the spin direction in photoexcited states. These results permit the tuning of the spin polarization of optically excited electrons in solids with strong spin–orbit interaction. PMID:28232721

  10. On local invariants of pure three-qubit states

    NASA Astrophysics Data System (ADS)

    Sudbery, Anthony

    2001-01-01

    We study invariants of three-qubit states under local unitary transformations, i.e. functions on the space of entanglement types, which is known to have dimension six. We show that there is no set of six algebraically independent polynomial invariants of degree ≤ 6, and find such a set with maximum degree eight. We describe an intrinsic definition of a canonical state on each orbit, and discuss the (non-polynomial) invariants associated with it.

  11. Synergic on/off Photoswitching Spin State and Magnetic Coupling between Spin Crossover Centers.

    PubMed

    Wang, Jun-Li; Liu, Qiang; Meng, Yin-Shan; Zheng, Hui; Zhu, Hai-Lang; Shi, Quan; Liu, Tao

    2017-09-05

    The existence of a correlation between spin crossover and dielectric properties is a hot topic in the field of multiresponse materials, which has potential applications in the memory devices, switches, and sensors. One formidable challenge is the simultaneous and rapid on/off switching of spin states of the spin carriers and magnetic coupling between them, which is crucial for both reversible photomagnetic behavior and variations in dielectric properties. Here, we report a dinuclear Fe(II) spin crossover complex, wherein each Fe(II) center exhibits an interconversion between Fe(II)HS (HS = high-spin) and Fe(II)LS (LS = low-spin) achieved upon heating and cooling. Moreover, the spin state of respective Fe(II) ions and the antiferromagnetic interaction between them can be switched bidirectionally under alternating irradiation with 532 and 808 nm light, resulting in interconversion between paramagnetic and diamagnetic properties. Interestingly, the spin crossover can also induce variations in dielectric tensors. This result provides a strategy to simultaneously and bidirectionally switch spin state, magnetic coupling, and dielectric properties using external stimuli.

  12. Spin-polarized surface resonances accompanying topological surface state formation

    SciTech Connect

    Jozwiak, Chris; Sobota, Jonathan A.; Gotlieb, Kenneth; Kemper, Alexander F.; Rotundu, Costel R.; Birgeneau, Robert J.; Hussain, Zahid; Lee, Dung -Hai; Shen, Zhi -Xun; Lanzara, Alessandra

    2016-10-14

    Topological insulators host spin-polarized surface states born out of the energetic inversion of bulk bands driven by the spin-orbit interaction. Here we discover previously unidentified consequences of band-inversion on the surface electronic structure of the topological insulator Bi2Se3. By performing simultaneous spin, time, and angle-resolved photoemission spectroscopy, we map the spin-polarized unoccupied electronic structure and identify a surface resonance which is distinct from the topological surface state, yet shares a similar spin-orbital texture with opposite orientation. Its momentum dependence and spin texture imply an intimate connection with the topological surface state. Calculations show these two distinct states can emerge from trivial Rashba-like states that change topology through the spin-orbit-induced band inversion. As a result, this work thus provides a compelling view of the coevolution of surface states through a topological phase transition, enabled by the unique capability of directly measuring the spin-polarized unoccupied band structure.

  13. Spin-polarized surface resonances accompanying topological surface state formation

    DOE PAGES

    Jozwiak, Chris; Sobota, Jonathan A.; Gotlieb, Kenneth; ...

    2016-10-14

    Topological insulators host spin-polarized surface states born out of the energetic inversion of bulk bands driven by the spin-orbit interaction. Here we discover previously unidentified consequences of band-inversion on the surface electronic structure of the topological insulator Bi2Se3. By performing simultaneous spin, time, and angle-resolved photoemission spectroscopy, we map the spin-polarized unoccupied electronic structure and identify a surface resonance which is distinct from the topological surface state, yet shares a similar spin-orbital texture with opposite orientation. Its momentum dependence and spin texture imply an intimate connection with the topological surface state. Calculations show these two distinct states can emerge frommore » trivial Rashba-like states that change topology through the spin-orbit-induced band inversion. As a result, this work thus provides a compelling view of the coevolution of surface states through a topological phase transition, enabled by the unique capability of directly measuring the spin-polarized unoccupied band structure.« less

  14. Spin-polarized surface resonances accompanying topological surface state formation

    NASA Astrophysics Data System (ADS)

    Jozwiak, Chris; Sobota, Jonathan A.; Gotlieb, Kenneth; Kemper, Alexander F.; Rotundu, Costel R.; Birgeneau, Robert J.; Hussain, Zahid; Lee, Dung-Hai; Shen, Zhi-Xun; Lanzara, Alessandra

    2016-10-01

    Topological insulators host spin-polarized surface states born out of the energetic inversion of bulk bands driven by the spin-orbit interaction. Here we discover previously unidentified consequences of band-inversion on the surface electronic structure of the topological insulator Bi2Se3. By performing simultaneous spin, time, and angle-resolved photoemission spectroscopy, we map the spin-polarized unoccupied electronic structure and identify a surface resonance which is distinct from the topological surface state, yet shares a similar spin-orbital texture with opposite orientation. Its momentum dependence and spin texture imply an intimate connection with the topological surface state. Calculations show these two distinct states can emerge from trivial Rashba-like states that change topology through the spin-orbit-induced band inversion. This work thus provides a compelling view of the coevolution of surface states through a topological phase transition, enabled by the unique capability of directly measuring the spin-polarized unoccupied band structure.

  15. Spin-polarized surface resonances accompanying topological surface state formation

    PubMed Central

    Jozwiak, Chris; Sobota, Jonathan A.; Gotlieb, Kenneth; Kemper, Alexander F.; Rotundu, Costel R.; Birgeneau, Robert J.; Hussain, Zahid; Lee, Dung-Hai; Shen, Zhi-Xun; Lanzara, Alessandra

    2016-01-01

    Topological insulators host spin-polarized surface states born out of the energetic inversion of bulk bands driven by the spin-orbit interaction. Here we discover previously unidentified consequences of band-inversion on the surface electronic structure of the topological insulator Bi2Se3. By performing simultaneous spin, time, and angle-resolved photoemission spectroscopy, we map the spin-polarized unoccupied electronic structure and identify a surface resonance which is distinct from the topological surface state, yet shares a similar spin-orbital texture with opposite orientation. Its momentum dependence and spin texture imply an intimate connection with the topological surface state. Calculations show these two distinct states can emerge from trivial Rashba-like states that change topology through the spin-orbit-induced band inversion. This work thus provides a compelling view of the coevolution of surface states through a topological phase transition, enabled by the unique capability of directly measuring the spin-polarized unoccupied band structure. PMID:27739428

  16. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6.

    PubMed

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X C; Zhang, Chi; Shi, Jing; Han, Wei

    2016-11-11

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin-momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin-momentum locking property of surface states of SmB6.

  17. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    NASA Astrophysics Data System (ADS)

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X. C.; Zhang, Chi; Shi, Jing; Han, Wei

    2016-11-01

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin-momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin-momentum locking property of surface states of SmB6.

  18. Spin-orbit coupling effect on the 23 Π state of 39K85Rb

    NASA Astrophysics Data System (ADS)

    Kim, Jin-Tae; Stolyarov, Andrey; Stwalley, William

    2013-05-01

    Recently we investigated the spin-orbit components (Ω = 0+, 0-, 1, and 2) of the 23 Π state of 39K85Rb by using experimental spectroscopy of ultracold molecules formed by photoassociation. The separations (Δ (EΩ = 1 -EΩ = 0) and Δ (EΩ = 2 -EΩ = 1)) between Ω components were unequal due to second-order perturbations by other electronic states. In the present work we investigate the spin-orbit coupling effect on the 2 3 Π state of 39K85Rb in the framework of 1st and 2nd order non-degenerate perturbation theory based on an ab initiomethod. Required potential energy curves and electronic spin-orbit coupling matrix elements are evaluated over a wide range of internuclear distance in the basis of the spin-averaged wavefunctions corresponding to the pure Hund's case (a) coupling scheme. We compare the experimental spin-orbit splittings of the 2 3 Π state with its ab initio counterparts, which agree well and elucidate the pronounced 2nd order perturbation effects caused by nearby electronic states.

  19. Spin-state transition of iron in (Ba0.5Sr0.5)(Fe0.8Zn0.2)O perovskite

    NASA Astrophysics Data System (ADS)

    Feldhoff, Armin; Martynczuk, Julia; Arnold, Mirko; Myndyk, Maxym; Bergmann, Ingo; Šepelák, Vladimir; Gruner, Wolfgang; Vogt, Ulrich; Hähnel, Angelika; Woltersdorf, Jörg

    2009-11-01

    The redox behavior of iron during heating of a high-performance perovskite for ceramic oxygen separation membranes was studied by combined electron energy-loss (EELS, esp. ELNES) and Mössbauer spectroscopical in situ methods. At room temperature, the iron in (Ba0.5Sr0.5)(Fe0.8Zn0.2)O (BSFZ) is in a mixed valence state of 75% Fe in the high-spin state and 25% Fe predominantly in the low-spin state. When heated to 900C, a slight reduction of iron is observed that increases the quantity of Fe species. However, the dominant occurrence is a gradual transition in the spin-state of trivalent iron from a mixed low-spin/high-spin to a pure high-spin configuration. In addition, a remarkable amount of hybridization is found in the Fe-O bonds that are highly polar rather than purely ionic. The coupled valence/spin-state transition correlates with anomalies in thermogravimetry and thermal expansion behavior observed by X-ray diffraction and dilatometry, respectively. Since the effective cationic radii depend not only on the valence but also on the spin-state, both have to be considered when estimating under which conditions a cubic perovskite will tolerate specific cations. It is concluded that an excellent phase stability of perovskite-based membrane materials demands a tailoring, which enables pure high-spin states under operational conditions, even if mixed valence states are present. The low spin-state transition temperature of BSFZ provides that all iron species are in a pure high-spin configuration already above ca. 500C making this ceramic highly attractive for intermediate temperature applications ( 500-800C).

  20. Localized States Influence Spin Transport in Epitaxial Graphene

    NASA Astrophysics Data System (ADS)

    Maassen, T.; van den Berg, J. J.; Huisman, E. H.; Dijkstra, H.; Fromm, F.; Seyller, T.; van Wees, B. J.

    2013-02-01

    We developed a spin transport model for a diffusive channel with coupled localized states that result in an effective increase of spin precession frequencies and a reduction of spin relaxation times in the system. We apply this model to Hanle spin precession measurements obtained on monolayer epitaxial graphene on SiC(0001). Combined with newly performed measurements on quasi-free-standing monolayer epitaxial graphene on SiC(0001) our analysis shows that the different values for the diffusion coefficient measured in charge and spin transport measurements on monolayer epitaxial graphene on SiC(0001) and the high values for the spin relaxation time can be explained by the influence of localized states arising from the buffer layer at the interface between the graphene and the SiC surface.

  1. Simulating spin-boson models with matrix product states

    NASA Astrophysics Data System (ADS)

    Wall, Michael; Safavi-Naini, Arghavan; Rey, Ana Maria

    2016-05-01

    The global coupling of few-level quantum systems (``spins'') to a discrete set of bosonic modes is a key ingredient for many applications in quantum science, including large-scale entanglement generation, quantum simulation of the dynamics of long-range interacting spin models, and hybrid platforms for force and spin sensing. In many situations, the bosons are integrated out, leading to effective long-range interactions between the spins; however, strong spin-boson coupling invalidates this approach, and spin-boson entanglement degrades the fidelity of quantum simulation of spin models. We present a general numerical method for treating the out-of-equilibrium dynamics of spin-boson systems based on matrix product states. While most efficient for weak coupling or small numbers of boson modes, our method applies for any spatial and operator dependence of the spin-boson coupling. In addition, our approach allows straightforward computation of many quantities of interest, such as the full counting statistics of collective spin measurements and quantum simulation infidelity due to spin-boson entanglement. We apply our method to ongoing trapped ion quantum simulator experiments in analytically intractable regimes. This work is supported by JILA-NSF-PFC-1125844, NSF-PIF- 1211914, ARO, AFOSR, AFOSR-MURI, and the NRC.

  2. Pure state consciousness and its local reduction to neuronal space

    NASA Astrophysics Data System (ADS)

    Duggins, A. J.

    2013-01-01

    The single neuronal state can be represented as a vector in a complex space, spanned by an orthonormal basis of integer spike counts. In this model a scalar element of experience is associated with the instantaneous firing rate of a single sensory neuron over repeated stimulus presentations. Here the model is extended to composite neural systems that are tensor products of single neuronal vector spaces. Depiction of the mental state as a vector on this tensor product space is intended to capture the unity of consciousness. The density operator is introduced as its local reduction to the single neuron level, from which the firing rate can again be derived as the objective correlate of a subjective element. However, the relational structure of perceptual experience only emerges when the non-local mental state is considered. A metric of phenomenal proximity between neuronal elements of experience is proposed, based on the cross-correlation function of neurophysiology, but constrained by the association of theoretical extremes of correlation/anticorrelation in inseparable 2-neuron states with identical and opponent elements respectively.

  3. Knitting distributed cluster-state ladders with spin chains

    SciTech Connect

    Ronke, R.; D'Amico, I.; Spiller, T. P.

    2011-09-15

    Recently there has been much study on the application of spin chains to quantum state transfer and communication. Here we discuss the utilization of spin chains (set up for perfect quantum state transfer) for the knitting of distributed cluster-state structures, between spin qubits repeatedly injected and extracted at the ends of the chain. The cluster states emerge from the natural evolution of the system across different excitation number sectors. We discuss the decohering effects of errors in the injection and extraction process as well as the effects of fabrication and random errors.

  4. Experimental Test of Residual Error-Disturbance Uncertainty Relations for Mixed SpinStates.

    PubMed

    Demirel, Bülent; Sponar, Stephan; Sulyok, Georg; Ozawa, Masanao; Hasegawa, Yuji

    2016-09-30

    The indeterminacy inherent in quantum measurements is an outstanding character of quantum theory, which manifests itself typically in the uncertainty principle. In the last decade, several universally valid forms of error-disturbance uncertainty relations were derived for completely general quantum measurements for arbitrary states. Subsequently, Branciard established a form that is optimal for spin measurements for some pure states. However, the bound in his inequality is not stringent for mixed states. One of the present authors recently derived a new bound tight in the corresponding mixed state case. Here, a neutron-optical experiment is carried out to investigate this new relation: it is tested whether error and disturbance of quantum measurements disappear or persist in mixing up the measured ensemble. The attainability of the new bound is experimentally observed, falsifying the tightness of Branciard's bound for mixed spin states.

  5. Determining asteroid spin states using radar speckles

    NASA Astrophysics Data System (ADS)

    Busch, Michael W.; Kulkarni, Shrinivas R.; Brisken, Walter; Ostro, Steven J.; Benner, Lance A. M.; Giorgini, Jon D.; Nolan, Michael C.

    2010-10-01

    Knowing the shapes and spin states of near-Earth asteroids is essential to understanding their dynamical evolution because of the Yarkovsky and YORP effects. Delay-Doppler radar imaging is the most powerful ground-based technique for imaging near-Earth asteroids and can obtain spatial resolution of <10 m, but frequently produces ambiguous pole direction solutions. A radar echo from an asteroid consists of a pattern of speckles caused by the interference of reflections from different parts of the surface. It is possible to determine an asteroid's pole direction by tracking the motion of the radar speckle pattern. Speckle tracking can potentially measure the poles of at least several radar targets each year, rapidly increasing the available sample of NEA pole directions. We observed the near-Earth asteroid 2008 EV5 with the Arecibo planetary radar and the Very Long Baseline Array in December 2008. By tracking the speckles moving from the Pie Town to Los Alamos VLBA stations, we have shown that EV5 rotates retrograde. This is the first speckle detection of a near-Earth asteroid.

  6. Decontaminating Solar Wind Samples with the Genesis Ultra-Pure Water Megasonic Wafer Spin Cleaner

    NASA Technical Reports Server (NTRS)

    Calaway, Michael J.; Rodriquez, M. C.; Allton, J. H.; Stansbery, E. K.

    2009-01-01

    The Genesis sample return capsule, though broken during the landing impact, contained most of the shattered ultra-pure solar wind collectors comprised of silicon and other semiconductor wafers materials. Post-flight analysis revealed that all wafer fragments were littered with surface particle contamination from spacecraft debris as well as soil from the impact site. This particulate contamination interferes with some analyses of solar wind. In early 2005, the Genesis science team decided to investigate methods for removing the surface particle contamination prior to solar wind analysis.

  7. Direct mapping of spin and orbital entangled wave functions under interband spin-orbit coupling of giant Rashba spin-split surface states

    NASA Astrophysics Data System (ADS)

    Noguchi, Ryo; Kuroda, Kenta; Yaji, K.; Kobayashi, K.; Sakano, M.; Harasawa, A.; Kondo, Takeshi; Komori, F.; Shin, S.

    2017-01-01

    We use spin- and angle-resolved photoemission spectroscopy (SARPES) combined with a polarization-variable laser and investigate the spin-orbit coupling effect under interband hybridization of Rashba spin-split states for the surface alloys Bi/Ag(111) and Bi/Cu(111). In addition to the conventional band mapping of photoemission for Rashba spin splitting, the different orbital and spin parts of the surface wave function are directly imaged into energy-momentum space. It is unambiguously revealed that the interband spin-orbit coupling modifies the spin and orbital character of the Rashba surface states leading to the enriched spin-orbital entanglement and the pronounced momentum dependence of the spin polarization. The hybridization thus strongly deviates the spin and orbital characters from the standard Rashba model. The complex spin texture under interband spin-orbit hybridization proposed by first-principles calculation is experimentally unraveled by SARPES with a combination of p - and s -polarized light.

  8. Valence and spin-state transition in cobaltates revisited by x-ray magnetic circular dichroism

    NASA Astrophysics Data System (ADS)

    Guillou, F.; Kummer, K.; Bréard, Y.; Hervé, L.; Hardy, V.

    2017-05-01

    The compounds ( Pr1 -ySmy)0.7Ca0.3CoO3 belong to a class of Pr-based cobaltates presenting a unique case of simultaneous valence (charge transfer between Pr and Co ions) and spin-state transition (of the Co3 + ions), hereafter referred to as VSST. The present study sheds light on the debated issues of the Co4 + and Co3 + spin states, by combining x-ray absorption spectroscopy (XAS) at Co and Pr edges and x-ray magnetic circular dichroism (XMCD) at Co L2 ,3 edges. XAS experiments at both L3 and M4 ,5 Pr edges attest to the appearance of Pr4 + below the VSST at T*=106 K , and allow a precise characterization of the evolution of the Co4 + content as a function of the temperature. XMCD at the Co L2 ,3 edges at 5 K, and in magnetic field up to 9 T, directly tackles the issue of the Co4 + spin state. It is found that the Co4 + ions are most likely in a low spin state, and experience ferromagnetic interactions at T ≪T* . On the basis of temperature dependent XMCD at 9 T, the fingerprint of the VSST on the Co moments is isolated, and found to be consistent with bulk magnetization data when accounting for the rare-earth contributions derived from reference samples. These temperature dependent XMCD data are used to characterize the evolutions of the various valence/spin state of the Co species involved in the VSST. It appears that the Co3 + moments above T* are not consistent with a pure intermediate spin state, whereas they can be well reproduced by considering a low/high spin mixture. Finally, these XMCD results are compared to those derived from fitting of the XAS spectra recorded in zero field at various temperatures.

  9. Local unitary invariants for N-qubit pure states

    SciTech Connect

    Sharma, S. Shelly; Sharma, N. K.

    2010-11-15

    The concept of negativity font, a basic unit of multipartite entanglement, is introduced. Transformation properties of determinants of negativity fonts under local unitary (LU) transformations are exploited to obtain relevant N-qubit polynomial invariants and construct entanglement monotones from first principles. It is shown that entanglement monotones that detect the entanglement of specific parts of the composite system may be constructed to distinguish between states with distinct types of entanglement. The structural difference between entanglement monotones for an odd and even number of qubits is brought out.

  10. Anticoherence of spin states with point-group symmetries

    NASA Astrophysics Data System (ADS)

    Baguette, D.; Damanet, F.; Giraud, O.; Martin, J.

    2015-11-01

    We investigate multiqubit permutation-symmetric states with maximal entropy of entanglement. Such states can be viewed as particular spin states, namely anticoherent spin states. Using the Majorana representation of spin states in terms of points on the unit sphere, we analyze the consequences of a point-group symmetry in their arrangement on the quantum properties of the corresponding state. We focus on the identification of anticoherent states (for which all reduced density matrices in the symmetric subspace are maximally mixed) associated with point-group-symmetric sets of points. We provide three different characterizations of anticoherence and establish a link between point symmetries, anticoherence, and classes of states equivalent through stochastic local operations with classical communication. We then investigate in detail the case of small numbers of qubits and construct infinite families of anticoherent states with point-group symmetry of their Majorana points, showing that anticoherent states do exist to arbitrary order.

  11. Charge-ordering cascade with spin-orbit Mott dimer states in metallic iridium ditelluride

    NASA Astrophysics Data System (ADS)

    Ko, K.-T.; Lee, H.-H.; Kim, D.-H.; Yang, J.-J.; Cheong, S.-W.; Eom, M. J.; Kim, J. S.; Gammag, R.; Kim, K.-S.; Kim, H.-S.; Kim, T.-H.; Yeom, H.-W.; Koo, T.-Y.; Kim, H.-D.; Park, J.-H.

    2015-06-01

    Spin-orbit coupling results in technologically-crucial phenomena underlying magnetic devices like magnetic memories and energy-efficient motors. In heavy element materials, the strength of spin-orbit coupling becomes large to affect the overall electronic nature and induces novel states such as topological insulators and spin-orbit-integrated Mott states. Here we report an unprecedented charge-ordering cascade in IrTe2 without the loss of metallicity, which involves localized spin-orbit Mott states with diamagnetic Ir4+-Ir4+ dimers. The cascade in cooling, uncompensated in heating, consists of first order-type consecutive transitions from a pure Ir3+ phase to Ir3+-Ir4+ charge-ordered phases, which originate from Ir 5d to Te 5p charge transfer involving anionic polymeric bond breaking. Considering that the system exhibits superconductivity with suppression of the charge order by doping, analogously to cuprates, these results provide a new electronic paradigm of localized charge-ordered states interacting with itinerant electrons through large spin-orbit coupling.

  12. Foucault's pendulum, a classical analog for the electron spin state

    NASA Astrophysics Data System (ADS)

    Linck, Rebecca A.

    Spin has long been regarded as a fundamentally quantum phenomena that is incapable of being described classically. To bridge the gap and show that aspects of spin's quantum nature can be described classically, this work uses a classical Lagrangian based on the coupled oscillations of Foucault's pendulum as an analog for the electron spin state in an external magnetic field. With this analog it is possible to demonstrate that Foucault's pendulum not only serves as a basis for explaining geometric phase, but is also a basis for reproducing a broad range of behavior from Zeeman-like frequency splitting to precession of the spin state. By demonstrating that unmeasured electron spin states can be fully described in classical terms, this research opens the door to using the tools of classical physics to examine an inherently quantum phenomenon.

  13. Electronic spin state of iron in lower mantle perovskite

    PubMed Central

    Li, Jie; Struzhkin, Viktor V.; Mao, Ho-kwang; Shu, Jinfu; Hemley, Russell J.; Fei, Yingwei; Mysen, Bjorn; Dera, Przemek; Prakapenka, Vitali; Shen, Guoyin

    2004-01-01

    The electronic spin state of iron in lower mantle perovskite is one of the fundamental parameters that governs the physics and chemistry of the most voluminous and massive shell in the Earth. We present experimental evidence for spin-pairing transition in aluminum-bearing silicate perovskite (Mg,Fe)(Si,Al)O3 under the lower mantle pressures. Our results demonstrate that as pressure increases, iron in perovskite transforms gradually from the initial high-spin state toward the final low-spin state. At 100 GPa, both aluminum-free and aluminum-bearing samples exhibit a mixed spin state. The residual magnetic moment in the aluminum-bearing perovskite is significantly higher than that in its aluminum-free counterpart. The observed spin evolution with pressure can be explained by the presence of multiple iron species and the occurrence of partial spin-paring transitions in the perovskite. Pressure-induced spin-pairing transitions in the perovskite would have important bearing on the magnetic, thermoelastic, and transport properties of the lower mantle, and on the distribution of iron in the Earth's interior. PMID:15377786

  14. Entanglement of Spin States in 15N@C60

    NASA Astrophysics Data System (ADS)

    Scherer, W.; Weidinger, A.; Mehring, M.

    2004-09-01

    The endohedral fullerene 15N@C60 comprises an electron spin S = 3/2 coupled to a nuclear spin I = 1/2 and is therefore ideally suited for experimental testing of basic properties of quantum mechanics. We will show that the 15N@C60 molecule represents a multi qubit system where different kinds of entangled states can be generated.

  15. Spin-adapted matrix product states and operators

    NASA Astrophysics Data System (ADS)

    Keller, Sebastian; Reiher, Markus

    2016-04-01

    Matrix product states (MPSs) and matrix product operators (MPOs) allow an alternative formulation of the density matrix renormalization group algorithm introduced by White. Here, we describe how non-abelian spin symmetry can be exploited in MPSs and MPOs by virtue of the Wigner-Eckart theorem at the example of the spin-adapted quantum chemical Hamiltonian operator.

  16. Liquid-state nuclear spin comagnetometers.

    PubMed

    Ledbetter, M P; Pustelny, S; Budker, D; Romalis, M V; Blanchard, J W; Pines, A

    2012-06-15

    We discuss nuclear spin comagnetometers based on ultralow-field nuclear magnetic resonance in mixtures of miscible solvents, each rich in a different nuclear spin. In one version thereof, Larmor precession of protons and 19F nuclei in a mixture of thermally polarized pentane and hexafluorobenzene is monitored via a sensitive alkali-vapor magnetometer. We realize transverse relaxation times in excess of 20 s and suppression of magnetic field fluctuations by a factor of 3400. We estimate it should be possible to achieve single-shot sensitivity of about 5×10(-9)  Hz, or about 5×10(-11)  Hz in ≈1 day of integration. In a second version, spin precession of protons and 129Xe nuclei in a mixture of pentane and hyperpolarized liquid xenon is monitored using superconducting quantum interference devices. Application to spin-gravity experiments, electric dipole moment experiments, and sensitive gyroscopes is discussed.

  17. Liquid-State Nuclear Spin Comagnetometers

    NASA Astrophysics Data System (ADS)

    Ledbetter, M. P.; Pustelny, S.; Budker, D.; Romalis, M. V.; Blanchard, J. W.; Pines, A.

    2012-06-01

    We discuss nuclear spin comagnetometers based on ultralow-field nuclear magnetic resonance in mixtures of miscible solvents, each rich in a different nuclear spin. In one version thereof, Larmor precession of protons and F19 nuclei in a mixture of thermally polarized pentane and hexafluorobenzene is monitored via a sensitive alkali-vapor magnetometer. We realize transverse relaxation times in excess of 20 s and suppression of magnetic field fluctuations by a factor of 3400. We estimate it should be possible to achieve single-shot sensitivity of about 5×10-9Hz, or about 5×10-11Hz in ≈1 day of integration. In a second version, spin precession of protons and Xe129 nuclei in a mixture of pentane and hyperpolarized liquid xenon is monitored using superconducting quantum interference devices. Application to spin-gravity experiments, electric dipole moment experiments, and sensitive gyroscopes is discussed.

  18. Foucault's Pendulum, Analog for an Electron Spin State

    NASA Astrophysics Data System (ADS)

    Linck, Rebecca

    2012-11-01

    The classical Lagrangian that describes the coupled oscillations of Foucault's pendulum presents an interesting analog to an electron's spin state in an external magnetic field. With a simple modification, this classical Lagrangian yields equations of motion that directly map onto the Schrodinger-Pauli Equation. This analog goes well beyond the geometric phase, reproducing a broad range of behavior from Zeeman-like frequency splitting to precession of the spin state. By demonstrating that unmeasured spin states can be fully described in classical terms, this research opens the door to using the tools of classical physics to examine an inherently quantum phenomenon.

  19. Simulating generic spin-boson models with matrix product states

    NASA Astrophysics Data System (ADS)

    Wall, Michael L.; Safavi-Naini, Arghavan; Rey, Ana Maria

    2016-11-01

    The global coupling of few-level quantum systems ("spins") to a discrete set of bosonic modes is a key ingredient for many applications in quantum science, including large-scale entanglement generation, quantum simulation of the dynamics of long-range interacting spin models, and hybrid platforms for force and spin sensing. We present a general numerical framework for treating the out-of-equilibrium dynamics of such models based on matrix product states. Our approach applies for generic spin-boson systems: it treats any spatial and operator dependence of the two-body spin-boson coupling and places no restrictions on relative energy scales. We show that the full counting statistics of collective spin measurements and infidelity of quantum simulation due to spin-boson entanglement, both of which are difficult to obtain by other techniques, are readily calculable in our approach. We benchmark our method using a recently developed exact solution for a particular spin-boson coupling relevant to trapped ion quantum simulators. Finally, we show how decoherence can be incorporated within our framework using the method of quantum trajectories, and study the dynamics of an open-system spin-boson model with spatially nonuniform spin-boson coupling relevant for trapped atomic ion crystals in the presence of molecular ion impurities.

  20. All-electric control of single atom spin states

    NASA Astrophysics Data System (ADS)

    Otte, Sander

    2011-03-01

    The quantum state of a single spin is a great candidate for forming a qubit. Spin systems in various forms are considered for the task, ranging from electrons trapped in artificial quantum dots to magnetic dopants in semiconductors and diamond. In this talk I will review recent progress towards controlling the spins of individual atoms on a surface through local access with an STM probe tip: an intriguing approach in view of the possibility to rearrange the atoms at will so as to build multi-atom structures. Magnetic d-metal atoms, separated from a metal substrate by a thin decoupling layer, are studied through inelastic electron tunneling spectroscopy (IETS): a tool by which transition energies of the spin state can be accurately followed. By addressing the atoms with a spin-filtered probe tip, controlled excitations or de-excitations can be made, effectively pumping the spin into a magnetization direction of choice. In a more recent experiment, spin pumping is performed in short pulses, opening up ways to control atomic spins in the time domain. I will discuss avenues to further develop this technique, eventually leading to coherent control of an atomic spin qubit.

  1. The Governance and Organizational Affiliation of Regional Educational Service Agencies: Arms of the State Education Agency, Pure Creatures of Constituent Local Districts, or Pure Special District Governments?

    ERIC Educational Resources Information Center

    Stephens, E. Robert

    Focusing on one of the most critical and complex aspects of the concept of the regional educational service agency (RESA), the paper questions whether RESA's should be an arm of the state educational agency, pure creatures of constituent local school districts, or pure special district governments. The critical dimensions of the issue being…

  2. Reduced quantum dynamics with initial system-environment correlations characterized by pure Markov states

    NASA Astrophysics Data System (ADS)

    Türkmen, A.; Verçin, A.; Yılmaz, S.

    2016-09-01

    Any tripartite state which saturates the strong subadditivity relation for the quantum entropy is defined as the Markov state. A tripartite pure state describing an open system, its environment, and their purifying system is a pure Markov state if and only if the bipartite marginal state of the purifying system and environment is a product state. It has been shown that as long as the purification of the input system-environment state is a pure Markov state, the reduced dynamics of the open system can be described, on the support of the initial system state, by a quantum channel for every joint unitary evolution of the system-environment composite even in the presence of initial correlations. Entanglement, discord, and classical correlations of the initial system-environment states implied by the pure Markov states are analyzed and it has been shown that all these correlations are entirely specified by the entropy of environment. Some implications concerning perfect quantum error correction procedure and quantum Markovian dynamics are presented.

  3. Photocreating supercooled spiral-spin states in a multiferroic manganite

    NASA Astrophysics Data System (ADS)

    Sheu, Y. M.; Ogawa, N.; Kaneko, Y.; Tokura, Y.

    2016-08-01

    We demonstrate that the dynamics of the a b -spiral-spin order in a magnetoelectric multiferroic Eu0.55Y0.45MnO3 can be unambiguously probed through optical second harmonic signals, generated via spin-induced ferroelectric polarization. In the case of weak excitation, the ferroelectric and the spiral-spin order remains interlocked, both relaxing through spin-lattice relaxation in the nonequilibrium state. When the additional optical pulse illuminating the sample is intense enough to induce a local phase transition thermally, the system creates a metastable state of the b c -spiral-spin order (with the electric polarization P ∥c ) via supercooling across the first-order phase transition between the a b and b c spiral. The supercooled state of the b c -spiral spin is formed in the thermodynamical ground state of the a b spiral (P ∥a ), displaying a prolonged lifetime with strong dependence on the magnetic field along the a axis. The observed phenomena provide a different paradigm for photoswitching between the two distinct multiferroic states, motivating further research into a direct observation of the photocreated supercooled b c -spiral spin in multiferroic manganites.

  4. Geometric characterization of separability and entanglement in pure Gaussian states by single-mode unitary operations

    NASA Astrophysics Data System (ADS)

    Adesso, Gerardo; Giampaolo, Salvatore M.; Illuminati, Fabrizio

    2007-10-01

    We present a geometric approach to the characterization of separability and entanglement in pure Gaussian states of an arbitrary number of modes. The analysis is performed adapting to continuous variables a formalism based on single subsystem unitary transformations that has been recently introduced to characterize separability and entanglement in pure states of qubits and qutrits [S. M. Giampaolo and F. Illuminati, Phys. Rev. A 76, 042301 (2007)]. In analogy with the finite-dimensional case, we demonstrate that the 1×M bipartite entanglement of a multimode pure Gaussian state can be quantified by the minimum squared Euclidean distance between the state itself and the set of states obtained by transforming it via suitable local symplectic (unitary) operations. This minimum distance, corresponding to a , uniquely determined, extremal local operation, defines an entanglement monotone equivalent to the entropy of entanglement, and amenable to direct experimental measurement with linear optical schemes.

  5. Geometric characterization of separability and entanglement in pure Gaussian states by single-mode unitary operations

    SciTech Connect

    Adesso, Gerardo; Giampaolo, Salvatore M.; Illuminati, Fabrizio

    2007-10-15

    We present a geometric approach to the characterization of separability and entanglement in pure Gaussian states of an arbitrary number of modes. The analysis is performed adapting to continuous variables a formalism based on single subsystem unitary transformations that has been recently introduced to characterize separability and entanglement in pure states of qubits and qutrits [S. M. Giampaolo and F. Illuminati, Phys. Rev. A 76, 042301 (2007)]. In analogy with the finite-dimensional case, we demonstrate that the 1xM bipartite entanglement of a multimode pure Gaussian state can be quantified by the minimum squared Euclidean distance between the state itself and the set of states obtained by transforming it via suitable local symplectic (unitary) operations. This minimum distance, corresponding to a, uniquely determined, extremal local operation, defines an entanglement monotone equivalent to the entropy of entanglement, and amenable to direct experimental measurement with linear optical schemes.

  6. Destination state screening of active spaces in spin dynamics simulations

    NASA Astrophysics Data System (ADS)

    Krzystyniak, M.; Edwards, Luke J.; Kuprov, Ilya

    2011-06-01

    We propose a novel avenue for state space reduction in time domain Liouville space spin dynamics simulations, using detectability as a selection criterion - only those states that evolve into or affect other detectable states are kept in the simulation. This basis reduction procedure (referred to as destination state screening) is formally exact and can be applied on top of the existing state space restriction techniques. As demonstrated below, in many cases this results in further reduction of matrix dimension, leading to considerable acceleration of many spin dynamics simulation types. Destination state screening is implemented in the latest version of the Spinach library (http://spindynamics.org).

  7. An Ising spin state explanation for financial asset allocation

    NASA Astrophysics Data System (ADS)

    Horvath, Philip A.; Roos, Kelly R.; Sinha, Amit

    2016-03-01

    We build on the developments in the application of statistical mechanics, notably the identity of the spin degree of freedom in the Ising model, to explain asset price dynamics in financial markets with a representative agent. Specifically, we consider the value of an individual spin to represent the proportional holdings in various assets. We use partial moment arguments to identify asymmetric reactions to information and develop an extension of a plunging and dumping model. This unique identification of the spin is a relaxation of the conventional discrete state limitation on an Ising spin to accommodate a new archetype in Ising model-finance applications wherein spin states may take on continuous values, and may evolve in time continuously, or discretely, depending on the values of the partial moments.

  8. Theory of unconventional spin states in surfaces with non-Rashba spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Nakajin, Kokin; Murakami, Shuichi

    2015-06-01

    Surface states in Tl /Si (111 )-(1 ×1 ) and β -Bi /Si (111 )-(√{3 }×√{3 } ) show non-Rashba-type spin splitting. We study spin-transport properties in these surface states. First, we construct tight-binding Hamiltonians for Tl/Si and Bi/Si surfaces, which respect crystallographic symmetries. As a result, we find specific terms in the Tl/Si surface Hamiltonian responsible for non-Rashba spin splitting. Using this model, we calculate current-induced spin polarization in the Tl/Si Hamiltonian in order to see the effect of non-Rashba spin-orbit interaction. We found that the induced spin polarization is in plane and perpendicular to the current, which is consequently the same with Rashba systems. We find that it follows from crystallographic symmetries. Furthermore, we numerically find bound states at the junction between two surface regions which have different signs of the spin-orbit interaction parameters in the Bi/Si system and in the Tl/Si system. We explain these numerical results with the results of our analytical calculations.

  9. Do Spin State and Spin Density Affect Hydrogen Atom Transfer Reactivity?

    PubMed Central

    Saouma, Caroline T.

    2013-01-01

    The prevalence of hydrogen atom transfer (HAT) reactions in chemical and biological systems has prompted much interest in establishing and understanding the underlying factors that enable this reactivity. Arguments have been advanced that the electronic spin state of the abstractor and/or the spin-density at the abstracting atom are critical for HAT reactivity. This is consistent with the intuition derived from introductory organic chemistry courses. Herein we present an alternative view on the role of spin state and spin-density in HAT reactions. After a brief introduction, the second section introduces a new and simple fundamental kinetic analysis, which shows that unpaired spin cannot be the dominant effect. The third section examines published computational studies of HAT reactions, which indicates that the spin state affects these reactions indirectly, primarily via changes in driving force. The essay concludes with a broader view of HAT reactivity, including indirect effects of spin and other properties on reactivity. It is suggested that some of the controversy in this area may arise from the diversity of HAT reactions and their overlap with proton-coupled electron transfer (PCET) reactions. PMID:24416504

  10. Probing photoinduced spin states in spin-crossover molecules with neutron scattering

    NASA Astrophysics Data System (ADS)

    Ridier, K.; Craig, G. A.; Damay, F.; Fennell, T.; Murrie, M.; Chaboussant, G.

    2017-03-01

    We report a neutron-scattering investigation of the spin-crossover compound [Fe (ptz) 6] (BF4)2 , which undergoes an abrupt thermal spin transition from high spin (HS), S =2 , to low spin (LS), S =0 , around 135 K. The HS magnetic state can be restored at low temperature under blue/green light irradiation. We have developed a specially designed optical setup for neutron scattering to address the magnetic properties of the light-induced HS state. By using neutron diffraction, we demonstrate that significant HS/LS ratios (of up to 60%) can be obtained with this experimental setup on a sample volume considered large (400 mg), while a complete recovery of the LS state is achieved using near-infrared light. Finally, with inelastic neutron scattering (INS) we have observed magnetic transitions arising from the photo-induced metastable HS S =2 state split by crystal-field and spin-orbit coupling. We interpret the INS data assuming a spin-only model with a zero-field splitting of the S =2 ground state. The obtained parameters are D ≈-1.28 ±0.03 meV and |E |≈0.08 ±0.03 meV. The present results show that in situ magnetic inelastic neutron-scattering investigations on a broad range of photomagnetic materials are now possible.

  11. High spin states in {sup 139}Pm

    SciTech Connect

    Dhal, A.; Sinha, R. K.; Chaturvedi, L.; Agarwal, P.; Kumar, S.; Jain, A. K.; Kumar, R.; Govil, I. M.; Mukhopadhyay, S.; Chakraborty, A.; Krishichayan; Ray, S.; Ghugre, S. S.; Sinha, A. K.; Kumar, R.; Singh, R. P.; Muralithar, S.; Bhowmik, R. K.; Pancholi, S. C.; Gupta, J. B.

    2009-07-15

    The odd mass nucleus {sup 139}Pm has been studied to high spins through the {sup 116}Cd({sup 27}Al,4n){sup 139}Pm reaction at an incident beam energy of 120 MeV. The de-exciting {gamma}-rays were detected using an array of 12 Compton suppressed Ge detectors. A total of 46 new levels have been proposed in the present work as a result of the observation of 60 new {gamma}-rays. Four new bands including a {delta}J=1 sequence have been identified and all the earlier reported bands, other than the yrast band, have been extended to higher spins and excitation energy. The spin assignments for most of the newly reported levels have been made using the observed coincidence angular anisotropy. Tilted axis cranking calculations support the interpretation of two of the observed magnetic dipole sequences as examples of magnetic rotational bands.

  12. Theory of resonance fluorescence from a solid-state cavity QED system: Effects of pure dephasing

    SciTech Connect

    Koshino, Kazuki

    2011-09-15

    We theoretically analyze the resonance fluorescence of a solid-state cavity quantum electrodynamics (QED) system that consists of a quantum dot and a cavity. We clarify the effects of pure dephasing by investigating the elastic and inelastic scattering probabilities, the fluorescence power spectrum, and the energy exchange with the environment. Pure dephasing interactions with the environment both enhance nonresonant coupling between the dot and the cavity and enable the pump light to continuously absorb energy from the environment under appropriate conditions.

  13. Electronic spin state of iron in lower mantle perovskite

    SciTech Connect

    Li, J.; Struzhkin, V.; Mao, H.-k.; Shu, J.; Hemley, R.; Fei, Y.; Mysen, B.; Dera, P.; Parapenka, V.; Shen, G.

    2010-11-16

    The electronic spin state of iron in lower mantle perovskite is one of the fundamental parameters that governs the physics and chemistry of the most voluminous and massive shell in the Earth. We present experimental evidence for spin-pairing transition in aluminum-bearing silicate perovskite (Mg,Fe)(Si,Al)O{sub 3} under the lower mantle pressures. Our results demonstrate that as pressure increases, iron in perovskite transforms gradually from the initial high-spin state toward the final low-spin state. At 100 GPa, both aluminum-free and aluminum-bearing samples exhibit a mixed spin state. The residual magnetic moment in the aluminum-bearing perovskite is significantly higher than that in its aluminum-free counterpart. The observed spin evolution with pressure can be explained by the presence of multiple iron species and the occurrence of partial spin-paring transitions in the perovskite. Pressure-induced spin-pairing transitions in the perovskite would have important bearing on the magnetic, thermoelastic, and transport properties of the lower mantle, and on the distribution of iron in the Earth's interior. The lower mantle constitutes more than half of the Earth's interior by volume (1), and it is believed to consist predominantly (80-100%) of (Mg,Fe)(Si,Al)O{sub 3} perovskite (hereafter called perovskite), with up to 20% (Mg,Fe)O ferropericlase (2). The electronic spin state of iron has direct influence on the physical properties and chemical behavior of its host phase. Hence, knowledge on the spin state of iron is important for the interpretation of seismic observations, geochemical modeling, and geodynamic simulation of the Earth's deep interior (3, 4). Crystal field theory (4, 5) and band theory (6) predicted that a high-spin to low-spin transition would occur as a result of compression. To date, no experimental data exist on the spin sate of iron in Al-bearing perovskite. To detect possible spinpairing transition of iron in perovskite under the lower mantle

  14. Ground states of the spin-1 Bose-Hubbard model.

    PubMed

    Katsura, Hosho; Tasaki, Hal

    2013-03-29

    We prove basic theorems about the ground states of the S=1 Bose-Hubbard model. The results are quite universal and depend only on the coefficient U2 of the spin-dependent interaction. We show that the ground state exhibits saturated ferromagnetism if U2<0, is spin-singlet if U2>0, and exhibits "SU(3)-ferromagnetism" if U2=0, and completely determine the degeneracy in each region.

  15. High-spin states in the 97Tc nucleus

    NASA Astrophysics Data System (ADS)

    Bucurescu, D.; Gadea, A.; Căta-Danil, Ghe.; Căta-Danil, I.; Ivaşcu, M.; Mărginean, N.; Rusu, C.; Stroe, L.; Ur, C. A.

    High-spin states in the 97Tc nucleus have been studied by in-beam γ-ray spectroscopy with the reaction 82Se(19F,4nγ) at 68 MeV incident energy. Excited states have been observed up to about 8 MeV excitation and spin 43/2ℎ. The observed level scheme is compared with results of shell model calculations.

  16. From spin glass to quantum spin liquid ground states in molybdate pyrochlores.

    PubMed

    Clark, L; Nilsen, G J; Kermarrec, E; Ehlers, G; Knight, K S; Harrison, A; Attfield, J P; Gaulin, B D

    2014-09-12

    We present new magnetic heat capacity and neutron scattering results for two magnetically frustrated molybdate pyrochlores: S=1 oxide Lu_{2}Mo_{2}O_{7} and S=1/2 oxynitride Lu_{2}Mo_{2}O_{5}N_{2}. Lu_{2}Mo_{2}O_{7} undergoes a transition to an unconventional spin glass ground state at T_{f}∼16  K. However, the preparation of the corresponding oxynitride tunes the nature of the ground state from spin glass to quantum spin liquid. The comparison of the static and dynamic spin correlations within the oxide and oxynitride phases presented here reveals the crucial role played by quantum fluctuations in the selection of a ground state. Furthermore, we estimate an upper limit for a gap in the spin excitation spectrum of the quantum spin liquid state of the oxynitride of Δ∼0.05  meV or Δ/|θ|∼0.004, in units of its antiferromagnetic Weiss constant θ∼-121  K.

  17. Spin-polarized state quantum filter used to measure spin-polarized state relaxation time and g-factor

    NASA Astrophysics Data System (ADS)

    Makarov, Vladimir I.; Khmelinskii, Igor

    2013-02-01

    A novel method for measurement of g-factor and spin-lattice relaxation time of spin-polarized states in nano-layers of different chemical nature was developed. This method is based on usage of spin-polarized state quantum filter, which was created and tested earlier [V. I. Makarov et al., J Appl. Phys. 110, 063717 (2011) and V. I. Makarov et al., J Appl. Phys. 112, 084310 (2012). The spin state parameters were measured in nanolayers of different materials (Fe, Au, and Si) in function of such experimental parameters as the layer thickness and temperature. The phenomenological model developed earlier for steady-state conditions was presently extended to include time dependence and successfully used in the data analysis. Qualitative models were proposed that explain the observed dependences, forming the basis for future theoretical developments.

  18. Lifetimes of high-spin states in 74Kr

    SciTech Connect

    Valiente-Dobon, J. J.; Svensson, C. E.; Grinyer, G. F.; Hyland, B.; Phillips, A. A.; Schumaker, M. A.; Steinhardt, T.; Eberth, J.; Stefanescu, I.; Thelen, O.; Afanasjev, A. V.; Ragnarsson, I.; Andreoiu, C.; Austin, R. A. E.; Carpenter, M. P.; Freeman, S. J.; Moore, F.; Mukherjee, G.; Seweryniak, D.; Dashdorj, D.

    2006-04-26

    High-spin states in {sub 36}{sup 74}Kr{sub 38} were studied using the 40Ca(40Ca,{alpha}2p)74Kr fusion evaporation reaction at a beam energy of 165 MeV with GAMMASPHERE and MICROBALL and at a beam energy of 185 MeV with EUROBALL and ISIS multi-detector arrays. Lifetimes of the high-spin states for the ground-state band and the favoured negative-parity band have been determined using the Doppler-shift attenuation method. The deduced transition quadrupole moments show a marginal decrease as a function of spin, suggesting that the rotational bands do not terminate at the maximum spin Imax.

  19. Dissipative entanglement of solid-state spins in diamond

    NASA Astrophysics Data System (ADS)

    Rao, D. D. Bhaktavatsala; Yang, Sen; Wrachtrup, Jörg

    2017-02-01

    Generating robust entanglement among solid-state spins is key for applications in quantum information processing and precision sensing. Here we show a dissipative approach to generate such entanglement among the hyperfine coupled electron nuclear spins using the rapid optical decay of electronic excited states. The combined dark state interference effects of the optical and microwave driving fields in the presence of spontaneous emission from the short-lived excited state leads to a dissipative formation of an entangled steady state. We show that the dissipative entanglement is generated for any initial state conditions of the spins and is resilient to external field fluctuations. We analyze the scheme for both continuous and pulsed driving fields in the presence of realistic noise sources.

  20. Quantum metrology with spin cat states under dissipation.

    PubMed

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-12-09

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms.

  1. Quantum metrology with spin cat states under dissipation

    NASA Astrophysics Data System (ADS)

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-12-01

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms.

  2. Quantum metrology with spin cat states under dissipation

    PubMed Central

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-01-01

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms. PMID:26647821

  3. Entangled Pure State Transformations via Local Operations Assisted by Finitely Many Rounds of Classical Communication.

    PubMed

    Spee, C; de Vicente, J I; Sauerwein, D; Kraus, B

    2017-01-27

    We consider generic pure n-qubit states and a general class of pure states of arbitrary dimensions and arbitrarily many subsystems. We characterize those states which can be reached from some other state via local operations assisted by finitely many rounds of classical communication (LOCC_{N}). For n qubits with n>3, we show that this set of states is of measure zero, which implies that the maximally entangled set is generically of full measure if restricted to the practical scenario of LOCC_{N}. Moreover, we identify a class of states for which any LOCC_{N} protocol can be realized via a concatenation of deterministic steps. We show, however, that in general there exist state transformations which require a probabilistic step within the protocol, which highlights the difference between bipartite and multipartite LOCC.

  4. Spin supercurrent, magnetization dynamics, and φ-state in spin-textured Josephson junctions

    NASA Astrophysics Data System (ADS)

    Kulagina, Iryna; Linder, Jacob

    2014-08-01

    The prospect of combining the dissipationless nature of superconducting currents with the spin polarization of magnetic materials is interesting with respect to exploring superconducting analogs of topics in spintronics. In order to accomplish this aim, it is pivotal to understand not only how such spin supercurrents can be created, but also how they interact dynamically with magnetization textures. In this paper, we investigate the appearance of a spin supercurrent and the resulting magnetization dynamics in a textured magnetic Josephson current by using three experimentally relevant models: (i) a superconductor∣ferromagnet∣superconductor (S∣F∣S) junction with spin-active interfaces, (ii) a S∣F1∣F2∣F3∣S Josephson junction with a ferromagnetic trilayer, and (iii) a Josephson junction containing a domain wall. In all of these cases, the supercurrent is spin polarized and exerts a spin-transfer torque on the ferromagnetic interlayers which causes magnetization dynamics. Using a scattering matrix formalism in the clean limit, we compute the Andreev bound states and resulting free energy of the system which in turn is used to solve the Landau-Lifshiftz-Gilbert equation. We compute both how the inhomogeneous magnetism influences the phase dependence of the charge supercurrent and the magnetization dynamics caused by the spin polarization of the supercurrent. Using a realistic experimental parameter set, we find that the spin supercurrent can induce magnetization switching that is controlled by the superconducting phase difference. Moreover, we demonstrate that the combined effect of chiral spin symmetry breaking of the system as a whole with interface scattering causes the systems above to act as phase batteries that may supply any superconducting phase difference φ in the ground state. Such a φ-junction is accompanied by an anomalous supercurrent appearing even at zero phase difference, and we demonstrate that the flow direction of this current is

  5. The structure of enumerated spin glass state spaces

    NASA Astrophysics Data System (ADS)

    Schubert, Sven; Hoffmann, Karl Heinz

    2006-02-01

    We enumerate the low energy part of the state space of an Ising spin glass using an efficient branch-and-bound algorithm. A coarse graining algorithm (NB-clustering) is employed to condense the inherent information to a system size which is treatable in computer simulations. The reduced state space still incorporates all ingredients necessary to simulate aging effects. We investigate its structure in detail and find that certain assumptions made in heuristical state space models which have been presented in the past to reproduce aging phenomena in spin glass experiments are indeed compatible with the data from the observed state spaces.

  6. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    SciTech Connect

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X. C.; Zhang, Chi; Shi, Jing; Han, Wei

    2016-11-11

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin–momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Moreover, the magnetic field angle dependence of the spin signal is consistent with spin–momentum locking property of surface states of SmB6.

  7. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    DOE PAGES

    Song, Qi; Mi, Jian; Zhao, Dan; ...

    2016-11-11

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin–momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observemore » the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Moreover, the magnetic field angle dependence of the spin signal is consistent with spin–momentum locking property of surface states of SmB6.« less

  8. Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6

    PubMed Central

    Song, Qi; Mi, Jian; Zhao, Dan; Su, Tang; Yuan, Wei; Xing, Wenyu; Chen, Yangyang; Wang, Tianyu; Wu, Tao; Chen, Xian Hui; Xie, X. C.; Zhang, Chi; Shi, Jing; Han, Wei

    2016-01-01

    There has been considerable interest in exploiting the spin degrees of freedom of electrons for potential information storage and computing technologies. Topological insulators (TIs), a class of quantum materials, have special gapless edge/surface states, where the spin polarization of the Dirac fermions is locked to the momentum direction. This spin–momentum locking property gives rise to very interesting spin-dependent physical phenomena such as the Edelstein and inverse Edelstein effects. However, the spin injection in pure surface states of TI is very challenging because of the coexistence of the highly conducting bulk states. Here, we experimentally demonstrate the spin injection and observe the inverse Edelstein effect in the surface states of a topological Kondo insulator, SmB6. At low temperatures when only surface carriers are present, a clear spin signal is observed. Furthermore, the magnetic field angle dependence of the spin signal is consistent with spin–momentum locking property of surface states of SmB6. PMID:27834378

  9. Deterministic LOCC transformation of three-qubit pure states and entanglement transfer

    NASA Astrophysics Data System (ADS)

    Tajima, Hiroyasu

    2013-02-01

    A necessary and sufficient condition of the possibility of a deterministic local operations and classical communication (LOCC) transformation of three-qubit pure states is given. The condition shows that the three-qubit pure states are a partially ordered set parametrized by five well-known entanglement parameters and a novel parameter; the five are the concurrences CAB, CAC, CBC, the tangle τABC and the fifth parameter J5 of Acín et al. (2000) Ref. [19], while the other new one is the entanglement charge Qe. The order of the partially ordered set is defined by the possibility of a deterministic LOCC transformation from a state to another state. In this sense, the present condition is an extension of Nielsen's work (Nielsen (1999) [14]) to three-qubit pure states. We also clarify the rules of transfer and dissipation of the entanglement which is caused by deterministic LOCC transformations. Moreover, the minimum number of times of measurements to reproduce an arbitrary deterministic LOCC transformation between three-qubit pure states is given.

  10. Optimal estimation of a physical observable's expectation value for pure states

    SciTech Connect

    Hayashi, A.; Horibe, M.; Hashimoto, T.

    2006-06-15

    We study the optimal way to estimate the quantum expectation value of a physical observable when a finite number of copies of a quantum pure state are presented. The optimal estimation is determined by minimizing the squared error averaged over all pure states distributed in a unitary invariant way. We find that the optimal estimation is 'biased' though the optimal measurement is given by successive projective measurements of the observable. The optimal estimate is not the sample average of observed data, but the arithmetic average of observed and ''default nonobserved'' data, with the latter consisting of all eigenvalues of the observable.

  11. Not all pure entangled states are useful for sub-shot-noise interferometry

    SciTech Connect

    Hyllus, Philipp; Smerzi, Augusto; Guehne, Otfried

    2010-07-15

    We investigate the connection between the shot-noise limit in linear interferometers and particle entanglement. In particular, we ask whether sub-shot-noise sensitivity can be reached with all pure entangled input states of N particles if they can be optimized with local operations. Results on the optimal local transformations allow us to show that for N=2 all pure entangled states can be made useful for sub-shot-noise interferometry while for N>2 this is not the case. We completely classify the useful entangled states available in a bosonic two-mode interferometer. We apply our results to several states, in particular to multiparticle singlet states and to cluster states. The latter turn out to be practically useless for sub-shot-noise interferometry. Our results are based on the Cramer-Rao bound and the Fisher information.

  12. Entangled states decoherence in coupled molecular spin clusters

    NASA Astrophysics Data System (ADS)

    Troiani, Filippo; Szallas, Attila; Bellini, Valerio; Affronte, Marco

    2010-03-01

    Localized electron spins in solid-state systems are widely investigated as potential building blocks of quantum devices and computers. While most efforts in the field have been focused on semiconductor low-dimensional structures, molecular antiferromagnets were recently recognized as alternative implementations of effective few-level spin systems. Heterometallic, Cr-based spin rings behave as effective spin-1/2 systems at low temperature and show long decoherence times [1]; besides, they can be chemically linked and magnetically coupled in a controllable fascion [2]. Here, we theoretically investigate the decoherence of the Bell states in such ring dimers, resulting from hyperfine interactions with nuclear spins. Based on a microscopic description of the molecules [3], we simulate the effect of inhomogeneous broadening, spectral diffusion and electron-nuclear entanglement on the electron-spin coherence, estimating the role of the different nuclei (and of possible chemical substitutions), as well as the effect of simple spin-echo sequences. References: [1] F. Troiani, et al., Phys. Rev. Lett. 94, 207208 (2005). [2] G. A. Timco, S: Carretta, F. Troiani et al., Nature Nanotech. 4, 173 (2009). [3] F. Troiani, V. Bellini, and M. Affronte, Phys. Rev. B 77, 054428 (2008).

  13. Spin states of the silicon vacancy in silicon carbide

    NASA Astrophysics Data System (ADS)

    Bockstedte, Michel; Schuetz, Felix

    2015-03-01

    SiC as a semi conductor fulfills all necessary requirements1 for implementing qubits via defect electron spins, such as the silicon vacancy, the di-vacancy or a complex of a silicon vacancy and a nitrogen impurity. The spin-selective fluorescence in contrast to the prototypical NV-center in diamond operates in the spectral range favorable for telecom applications.Spin-manipulation of the intrinsic centers was demonstrated even at room temperature.2,3 For the silicon vacancy in SiC inter system crossings (ISCs) from high to yet unknown low spin states govern the spin-relaxation. By DFT and a DFT-based multi-reference Hamiltonian we analyze the spin physics of the defect. In 4H SiC distinct luminescence lines are obtained for the inequivalent defect sites in agreement with experiment. Our result thus establishes an assignment of the lines to the sites. Owing to the spin (S=3/2) and a stronger electron-phonon coupling in the excited state, we find ISCs distinct from the NV-center.

  14. Economic and Deterministic Quantum Teleportation of Arbitrary Bipartite Pure and Mixed State with Shared Cluster Entanglement

    NASA Astrophysics Data System (ADS)

    Zhang, Binbin; Liu, Yu

    2009-09-01

    We present a novel protocol for teleportation of arbitrary bipartite pure and mixed state with shared cluster entanglement in this paper. By employing Bell-state measurement on the teleported state and the shared cluster state twice, a sender could transmit the arbitrary bipartite state to a distant receiver. We show the good feature of the cluster state channel, with which it can realize the deterministic teleportation rather than probabilistic one. Moreover, since we require less particles to be shared and need no auxiliary qubit in our protocol, it is more efficient and applicable than the previous schemes.

  15. Spin-pairing correlations and spin polarization of Majorana bound states in two-dimensional topological-insulator systems

    NASA Astrophysics Data System (ADS)

    Zhang, Kunhua; Zeng, Junjie; Ren, Yafei; Qiao, Zhenhua

    2017-08-01

    We demonstrate that a zero-energy Majorana bound state in a ferromagnetic insulator (FI)-superconductor (SC) junction formed on the edge of a two-dimensional topological insulator exhibits three types of spin-triplet pairing correlations, its spin-polarization direction is position independent in a ferromagnetic insulator, and demonstrates a spin-helix structure in a superconductor. These spin properties of Majorana bound states lead to anomalous selective equal-spin Andreev reflection. Similar behavior is found when the coupling between two Majorana bound states in a FI-SC-FI junction is invoked, though an additional weak spin-singlet pairing correlation is generated. These signatures can readily facilitate the experimental detection of spin-triplet correlations and spin polarization of Majorana bound states.

  16. Number of spin I states of identical particles

    SciTech Connect

    Zhao, Y.M.; Arima, A.

    2005-04-01

    In this article we study the enumeration of number (denoted as D{sub I}) of spin I states for fermions in a single-j shell and bosons with spin l. We show that D{sub I} can be enumerated by the reduction from SU(n+1) to SO(3). New regularities of D{sub I} are discerned. As an example of our new algorithm, we obtained analytical expressions of D{sub I} for four particles.

  17. High-spin states in the 96Tc nucleus

    NASA Astrophysics Data System (ADS)

    Bucurescu, D.; Căta-Danil, Gh.; Căta-Danil, I.; Ivaşcu, M.; Mărginean, N.; Rusu, C.; Stroe, L.; Ur, C. A.; Gizon, A.; Gizon, J.; Nyakó, B.; Timár, J.; Zolnai, L.; Boston, A. J.; Joss, D. T.; Paul, E. S.; Semple, A. T.; Parry, C. M.

    High-spin states in the 96Tc nucleus have been studied with the reactions 82Se(19F,5nγ) at 68 MeV and Zn(36S,αpxn) at 130 MeV. Two γ-ray cascades (irregular bandlike structures) have been observed up to an excitation energy of about 10 MeV and spin 21-22?.

  18. Lifetimes of High-Spin States in 76Kr

    NASA Astrophysics Data System (ADS)

    Valiente-Dobon, J. J.; Svensson, C. E.; O'Leary, C. D.; Ragnarsson, I.; Andreoiu, C.; Austin, R. A. E.; Carpenter, M. P.; Dashdorj, D.; Finlay, P.; Freeman, S. J.; Garrett, P. E.; Goergen, A.; Greene, J.; Grinyer, G. F.; Hyland, B.; Jenkins, D.; Johnston-Theasby, F.; Joshi, P.; Kelsall, N. S.; Macchiavelli, A. O.; Moore, F.; Mukherjee, G.; Phillips, A. A.; Reviol, W.; Sarantites, D.; Schumaker, M. A.; Seweryniak, D.; Smith, M. B.; Wadsworth, R.; Ward, D.

    2005-04-01

    High-spin states in 7636Kr40 have been populated in the 40Ca(40Ca,4p)76Kr fusion-evaporation reaction at a beam energy of 165 MeV, and studied using the GAMMASPHERE and MICROBALL multi-detector arrays. The ground-state band and two signature-split negative-parity bands of 76Kr have been extended to ˜ 30hbar. Lifetime measurements using the Doppler-shift attenuation method indicate that the transition quadrupole moment of these three bands decrease as they approach their maximum-spin states.

  19. One-Dimensional Edge States with Giant Spin Splitting in a Bismuth Thin Film

    NASA Astrophysics Data System (ADS)

    Takayama, A.; Sato, T.; Souma, S.; Oguchi, T.; Takahashi, T.

    2015-02-01

    To realize a one-dimensional (1D) system with strong spin-orbit coupling is a big challenge in modern physics, since the electrons in such a system are predicted to exhibit exotic properties unexpected from the 2D or 3D counterparts, while it was difficult to realize genuine physical properties inherent to the 1D system. We demonstrate the first experimental result that directly determines the purely 1D band structure by performing spin-resolved angle-resolved photoemission spectroscopy of Bi islands on a silicon surface that contains a metallic 1D edge structure with unexpectedly large Rashba-type spin-orbit coupling suggestive of the nontopological nature. We have also found a sizable out-of-plane spin polarization of the 1D edge state, consistent with our first-principles band calculations. Our result provides a new platform to realize exotic quantum phenomena at the 1D edge of the strong spin-orbit-coupling systems.

  20. Dressed-state resonant coupling between bright and dark spins in diamond.

    PubMed

    Belthangady, C; Bar-Gill, N; Pham, L M; Arai, K; Le Sage, D; Cappellaro, P; Walsworth, R L

    2013-04-12

    Under ambient conditions, spin impurities in solid-state systems are found in thermally mixed states and are optically "dark"; i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception in that the electronic spin states are "bright"; i.e., they can be polarized by optical pumping, coherently manipulated with spin-resonance techniques, and read out optically, all at room temperature. Here we demonstrate a scheme to resonantly couple bright NV electronic spins to dark substitutional-nitrogen (P1) electronic spins by dressing their spin states with oscillating magnetic fields. This resonant coupling mechanism can be used to transfer spin polarization from NV spins to nearby dark spins and could be used to cool a mesoscopic bath of dark spins to near-zero temperature, thus providing a resource for quantum information and sensing, and aiding studies of quantum effects in many-body spin systems.

  1. Entanglement in a solid-state spin ensemble.

    PubMed

    Simmons, Stephanie; Brown, Richard M; Riemann, Helge; Abrosimov, Nikolai V; Becker, Peter; Pohl, Hans-Joachim; Thewalt, Mike L W; Itoh, Kohei M; Morton, John J L

    2011-02-03

    Entanglement is the quintessential quantum phenomenon. It is a necessary ingredient in most emerging quantum technologies, including quantum repeaters, quantum information processing and the strongest forms of quantum cryptography. Spin ensembles, such as those used in liquid-state nuclear magnetic resonance, have been important for the development of quantum control methods. However, these demonstrations contain no entanglement and ultimately constitute classical simulations of quantum algorithms. Here we report the on-demand generation of entanglement between an ensemble of electron and nuclear spins in isotopically engineered, phosphorus-doped silicon. We combined high-field (3.4 T), low-temperature (2.9 K) electron spin resonance with hyperpolarization of the (31)P nuclear spin to obtain an initial state of sufficient purity to create a non-classical, inseparable state. The state was verified using density matrix tomography based on geometric phase gates, and had a fidelity of 98% relative to the ideal state at this field and temperature. The entanglement operation was performed simultaneously, with high fidelity, on 10(10) spin pairs; this fulfils one of the essential requirements for a silicon-based quantum information processor.

  2. Optimal state discrimination with an error margin of pure and mixed symmetric states: irreducible qudit and reducible qubit states

    NASA Astrophysics Data System (ADS)

    Jafarizadeh, M. A.; Mahmoudi, P.; Akhgar, D.; Faizi, E.

    2017-06-01

    Minimum error discrimination (MED) and Unambiguous discrimination (UD) are two common strategies for quantum state discrimination that can be modified by imposing a finite error margin on the error probability. Error margins 0 and 1 correspond to two common strategies. In this paper, for an arbitrary error margin m, the discrimination problem of equiprobable quantum symmetric states is analytically solved for four distinct cases. A generating set of irreducible and reducible representations of a subgroup of a unitary group are considered, separately, as unitary operators that produce one set of the symmetric states. In the irreducible case, for N≥slant d mixed and pure qudit states, one critical m which divides the parameter space into two domains is obtained. The number of critical values m in the reducible case is two, for both N mixed and pure qubit states. The reason for this difference between numbers of critical values m is explained. The optimal set of measurements and corresponding maximum success probability in fully analytical form are determined for all values of the error margin. The relationship between the amount of error that is imposed on error probability and geometrical situation of states with changes in rank of element corresponding to inconclusive result is determined. The behaviors of elements of measurement are explained geometrically in order to decrease the error probability in each domain. Furthermore, the problem of the discrimination with error margin among elements of two different sets of symmetric quantum states is studied. The number of critical values m is equivalent to one set in both reducible and irreducible cases. In addition, optimal measurements in each domain are obtained.

  3. Edge dynamics in a quantum spin Hall state: effects from Rashba spin-orbit interaction.

    PubMed

    Ström, Anders; Johannesson, Henrik; Japaridze, G I

    2010-06-25

    We analyze the dynamics of the helical edge modes of a quantum spin Hall state in the presence of a spatially nonuniform Rashba spin-orbit (SO) interaction. A randomly fluctuating Rashba SO coupling is found to open a scattering channel which causes localization of the edge modes for a weakly screened electron-electron (e-e) interaction. A periodic modulation of the SO coupling, with a wave number commensurate with the Fermi momentum, makes the edge insulating already at intermediate strengths of the e-e interaction. We discuss implications for experiments on edge state transport in a HgTe quantum well.

  4. DETERMINING TITAN'S SPIN STATE FROM CASSINI RADAR IMAGES

    SciTech Connect

    Stiles, Bryan W.; Hensley, Scott; Ostro, Steven J.; Callahan, Philip S.; Gim, Yonggyu; Hamilton, Gary; Johnson, William T. K.; West, Richard D.; Kirk, Randolph L.; Lee, Ella; Lorenz, Ralph D.; Allison, Michael D.; Iess, Luciano; Del Marmo, Paolo Perci

    2008-05-15

    For some 19 areas of Titan's surface, the Cassini RADAR instrument has obtained synthetic aperture radar (SAR) images during two different flybys. The time interval between flybys varies from several weeks to two years. We have used the apparent misregistration (by 10-30 km) of features between separate flybys to construct a refined model of Titan's spin state, estimating six parameters: north pole right ascension and declination, spin rate, and these quantities' first time derivatives We determine a pole location with right ascension of 39.48 degrees and declination of 83.43 degrees corresponding to a 0.3 degree obliquity. We determine the spin rate to be 22.5781 deg day{sup -1} or 0.001 deg day{sup -1} faster than the synchronous spin rate. Our estimated corrections to the pole and spin rate exceed their corresponding standard errors by factors of 80 and 8, respectively. We also found that the rate of change in the pole right ascension is -30 deg century{sup -1}, ten times faster than right ascension rate of change for the orbit normal. The spin rate is increasing at a rate of 0.05 deg day{sup -1} per century. We observed no significant change in pole declination over the period for which we have data. Applying our pole correction reduces the feature misregistration from tens of km to 3 km. Applying the spin rate and derivative corrections further reduces the misregistration to 1.2 km.

  5. Determining titan's spin state from cassini radar images

    USGS Publications Warehouse

    Stiles, B.W.; Kirk, R.L.; Lorenz, R.D.; Hensley, S.; Lee, E.; Ostro, S.J.; Allison, M.D.; Callahan, P.S.; Gim, Y.; Iess, L.; Del Marmo, P.P.; Hamilton, G.; Johnson, W.T.K.; West, R.D.

    2008-01-01

    For some 19 areas of Titan's surface, the Cassini RADAR instrument has obtained synthetic aperture radar (SAR) images during two different flybys. The time interval between flybys varies from several weeks to two years. We have used the apparent misregistration (by 10-30 km) of features between separate flybys to construct a refined model of Titan's spin state, estimating six parameters: north pole right ascension and declination, spin rate, and these quantities' first time derivatives We determine a pole location with right ascension of 39.48 degrees and declination of 83.43 degrees corresponding to a 0.3 degree obliquity. We determine the spin rate to be 22.5781 deg day -1 or 0.001 deg day-1 faster than the synchronous spin rate. Our estimated corrections to the pole and spin rate exceed their corresponding standard errors by factors of 80 and 8, respectively. We also found that the rate of change in the pole right ascension is -30 deg century-1, ten times faster than right ascension rate of change for the orbit normal. The spin rate is increasing at a rate of 0.05 deg day -1 per century. We observed no significant change in pole declination over the period for which we have data. Applying our pole correction reduces the feature misregistration from tens of km to 3 km. Applying the spin rate and derivative corrections further reduces the misregistration to 1.2 km. ?? 2008. The American Astronomical Society. All rights reserved.

  6. Spin-polarized local density of states in the vortex state of helical p -wave superconductors

    NASA Astrophysics Data System (ADS)

    Tanaka, Kenta K.; Ichioka, Masanori; Onari, Seiichiro

    2017-04-01

    Properties of the vortex state in helical p -wave superconductor are studied by the quasiclassical Eilenberger theory. We confirm the instability of the helical p -wave state at high fields and that the spin-polarized local density of states M (E ,r ) appears even when Knight shift does not change. This is because the vorticity couples to the chirality of up-spin pair or down-spin pair of the helical state. In order to identify the helical p -wave state at low fields, we investigate the structure of the zero-energy M (E =0 ,r ) in the vortex states, and also the energy spectra of M (E ,r ) .

  7. Striped spin liquid crystal ground state instability of kagome antiferromagnets.

    PubMed

    Clark, Bryan K; Kinder, Jesse M; Neuscamman, Eric; Chan, Garnet Kin-Lic; Lawler, Michael J

    2013-11-01

    The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities. This has been suggested as the reason why it does not emerge as the ground state in large-scale numerical calculations. However, previous attempts to observe these instabilities have failed. We report on the discovery of a projected BCS state with lower energy than the projected Dirac spin liquid state which provides new insight into the stability of the ground state of the kagome antiferromagnet. The new state has three remarkable features. First, it breaks spatial symmetry in an unusual way that may leave spinons deconfined along one direction. Second, it breaks the U(1) gauge symmetry down to Z(2). Third, it has the spatial symmetry of a previously proposed "monopole" suggesting that it is an instability of the Dirac spin liquid. The state described herein also shares a remarkable similarity to the distortion of the kagome lattice observed at low Zn concentrations in Zn-paratacamite and in recently grown single crystals of volborthite suggesting it may already be realized in these materials.

  8. Improved fair sampling of ground states in Ising spin glasses

    NASA Astrophysics Data System (ADS)

    Katzgraber, Helmut G.; Zhu, Zheng; Ochoa, Andrew J.

    2015-03-01

    Verifying that an optimization approach can sample all solutions that minimize a Hamiltonian is a stringent test for any newly-developed algorithm. While most solvers easily compute the minimum of a cost function for small to moderate input sizes, equiprobable sampling of all ground-state configurations (within Poissonian fluctuations) is much harder to obtain. Most notably, methods such as transverse-field quantum annealing fail in passing this test for certain highly-degenerate problems. Here we present an attempt to sample ground states for Ising spin glasses based on a combination of low-temperature parallel tempering Monte Carlo combined with the cluster algorithm by Houdayer. Because the latter is rejection free and obeys details balance, the ground-state manifold is efficiently sampled. We illustrate the approach for Ising spin glasses on the D-Wave Two quantum annealer topology, known as the Chimera graph, as well as two-dimensional Ising spin glasses.

  9. Phase-Tuned Entangled State Generation between Distant Spin Qubits

    NASA Astrophysics Data System (ADS)

    Stockill, R.; Stanley, M. J.; Huthmacher, L.; Clarke, E.; Hugues, M.; Miller, A. J.; Matthiesen, C.; Le Gall, C.; Atatüre, M.

    2017-07-01

    Quantum entanglement between distant qubits is an important feature of quantum networks. Distribution of entanglement over long distances can be enabled through coherently interfacing qubit pairs via photonic channels. Here, we report the realization of optically generated quantum entanglement between electron spin qubits confined in two distant semiconductor quantum dots. The protocol relies on spin-photon entanglement in the trionic Λ system and quantum erasure of the Raman-photon path information. The measurement of a single Raman photon is used to project the spin qubits into a joint quantum state with an interferometrically stabilized and tunable relative phase. We report an average Bell-state fidelity for |ψ(+)⟩ and |ψ(-)⟩ states of 61.6 ±2.3 % and a record-high entanglement generation rate of 7.3 kHz between distant qubits.

  10. Measurements of the spin-orbit interaction and Landé g factor in a pure-phase InAs nanowire double quantum dot in the Pauli spin-blockade regime

    SciTech Connect

    Wang, Jiyin; Huang, Shaoyun E-mail: syhuang@pku.edu.cn; Lei, Zijin; Pan, Dong; Zhao, Jianhua; Xu, H. Q. E-mail: syhuang@pku.edu.cn

    2016-08-01

    We demonstrate direct measurements of the spin-orbit interaction and Landé g factors in a semiconductor nanowire double quantum dot. The device is made from a single-crystal pure-phase InAs nanowire on top of an array of finger gates on a Si/SiO{sub 2} substrate and the measurements are performed in the Pauli spin-blockade regime. It is found that the double quantum dot exhibits a large singlet-triplet energy splitting of Δ{sub ST} ∼ 2.3 meV, a strong spin-orbit interaction of Δ{sub SO} ∼ 140 μeV, and a large and strongly level-dependent Landé g factor of ∼12.5. These results imply that single-crystal pure-phase InAs nanowires are desired semiconductor nanostructures for applications in quantum information technologies.

  11. Measurements of the spin-orbit interaction and Landé g factor in a pure-phase InAs nanowire double quantum dot in the Pauli spin-blockade regime

    NASA Astrophysics Data System (ADS)

    Wang, Jiyin; Huang, Shaoyun; Lei, Zijin; Pan, Dong; Zhao, Jianhua; Xu, H. Q.

    2016-08-01

    We demonstrate direct measurements of the spin-orbit interaction and Landé g factors in a semiconductor nanowire double quantum dot. The device is made from a single-crystal pure-phase InAs nanowire on top of an array of finger gates on a Si/SiO2 substrate and the measurements are performed in the Pauli spin-blockade regime. It is found that the double quantum dot exhibits a large singlet-triplet energy splitting of ΔST ˜ 2.3 meV, a strong spin-orbit interaction of ΔSO ˜ 140 μeV, and a large and strongly level-dependent Landé g factor of ˜12.5. These results imply that single-crystal pure-phase InAs nanowires are desired semiconductor nanostructures for applications in quantum information technologies.

  12. Approximate transformations of bipartite pure-state entanglement from the majorization lattice

    NASA Astrophysics Data System (ADS)

    Bosyk, G. M.; Sergioli, G.; Freytes, H.; Holik, F.; Bellomo, G.

    2017-05-01

    We study the problem of deterministic transformations of an initial pure entangled quantum state, | ψ > , into a target pure entangled quantum state, | ϕ > , by using local operations and classical communication (LOCC). A celebrated result of Nielsen (1999) gives the necessary and sufficient condition that makes this entanglement transformation process possible. Indeed, this process can be achieved if and only if the majorization relation ψ ≺ ϕ holds, where ψ and ϕ are probability vectors obtained by taking the squares of the Schmidt coefficients of the initial and target states, respectively. In general, this condition is not fulfilled. However, one can look for an approximate entanglement transformation. Vidal et al. (2000) have proposed a deterministic transformation using LOCC in order to obtain a target state |χopt > most approximate to | ϕ > in terms of maximal fidelity between them. Here, we show a strategy to deal with approximate entanglement transformations based on the properties of the majorization lattice. More precisely, we propose as approximate target state one whose Schmidt coefficients are given by the supremum between ψ and ϕ. Our proposal is inspired on the observation that fidelity does not respect the majorization relation in general. Remarkably enough, we find that for some particular interesting cases, like two-qubit pure states or the entanglement concentration protocol, both proposals are coincident.

  13. The integrated spintronic functionalities of an individual high-spin state spin-crossover molecule between graphene nanoribbon electrodes

    NASA Astrophysics Data System (ADS)

    Zhu, L.; Zou, F.; Gao, J. H.; Fu, Y. S.; Gao, G. Y.; Fu, H. H.; Wu, M. H.; Lü, J. T.; Yao, K. L.

    2015-08-01

    The spin-polarized transport properties of a high-spin-state spin-crossover molecular junction with zigzag-edge graphene nanoribbon electrodes have been studied using density functional theory combined with the nonequilibrium Green’s-function formalism. The molecular junction presents integrated spintronic functionalities such as negative differential resistance behavior, spin filter and the spin rectifying effect, associated with the giant magnetoresistance effect by tuning the external magnetic field. Furthermore, the transport properties are almost unaffected by the electrode temperature. The microscopic mechanism of these functionalities is discussed. These results represent a step toward multifunctional molecular spintronic devices on the level of the individual spin-crossover molecule.

  14. Spin blockade and coherent dynamics of high-spin states in a three-electron double quantum dot

    NASA Astrophysics Data System (ADS)

    Chen, Bao-Bao; Wang, Bao-Chuan; Cao, Gang; Li, Hai-Ou; Xiao, Ming; Guo, Guang-Can; Jiang, Hong-Wen; Hu, Xuedong; Guo, Guo-Ping

    2017-01-01

    Asymmetry in a three-electron double quantum dot (DQD) allows spin blockade, when spin-3/2 (quadruplet) states and spin-1/2 (doublet) states have different charge configurations. We have observed this DQD spin blockade near the (1,2)-(2,1) charge transition using a pulsed-gate technique and a charge sensor. We, then, use this spin blockade to detect Landau-Zener-Stückelberg interference and coherent oscillations between the spin quadruplet and doublet states. Such studies add to our understandings of coherence and control properties of three-spin states in a double dot, which, in turn, would benefit explorations into various qubit encoding schemes in semiconductor nanostructures.

  15. Nonlinear spin-torque microwave resonance near the loss of spin state stability

    NASA Astrophysics Data System (ADS)

    Popkov, A. F.; Kulagin, N. E.; Demin, G. D.

    2016-12-01

    The paper analyzes microwave resonant response of the spin-torque diode. The considered spin-torque diode is a magnetic tunnel junction with a nano-pillar structure. The magnetization of the free layer has a tilt caused by an action of the inclined magnetic field in the plane of the structure. Taking into account the effect of spin torque transfer we define stability regions of stationary states of magnetization in the free layer as a function of the azimuth angle of the magnetic field and bias DC current. Microwave volt-watt sensitivity of the spin diode for the obtained stationary states is calculated. It is shown that non-linear frequency shift of the resonance line width limits maximum sensitivity of the spin diode near the critical bias current corresponding to the point of the transition to the self-oscillating mode. Besides that, overlapping of frequency branches occurs in the resonant response as the critical point approach, which is different from the foldover effect in the nonlinear ferromagnetic resonance induced by an alternating magnetic field.

  16. Spin-Orbital Entangled States in Transition Metal Oxides

    NASA Astrophysics Data System (ADS)

    Oleś, Andrzej M.

    The phenomenon of spin-orbital entanglement which occurs in superexchange models for transition metal oxides is introduced and explained. We present its consequences in the RVO_3 Mott insulators, with R=La,Pr,\\cdots ,Yb,Lu, and show that entanglement occurs here in excited states of the spin-orbital d^2 model and determines: (i) the temperature dependence of low-energy optical spectral weight, (ii) the phase diagram of the RVO_3 perovskites, and (iii) the dimerization observed in the magnon excitations in YVO_3. Entangled ground states occur in two other model systems: (i) the bilayer d^9 (Kugel-Khomskii) model, and (ii) the d^1 model on the triangular frustrated lattice. In such cases even the predictions concerning the magnetic exchange constants based on the mean field decoupling of spin and orbital operators are incorrect. On the example of a single hole doped to a Mott insulator with coexisting antiferromagnetic and alternating t_{2g} orbital order we show that transport is hindered by spin-orbital excitations. It is suggested that spin-orbital entanglement in Mott insulators might be controlled by doping, leading to orbital disordered states with possible new opportunities for thermoelectric applications.

  17. Comprehensive analysis of quantum pure-state estimation for two-level systems

    SciTech Connect

    Bagan, E.; Monras, A.; Munoz-Tapia, R.

    2005-06-15

    Given N identical copies of the state of a quantum two-level system, we analyze its optimal estimation. We consider two situations: general pure states and (pure) states restricted to lie on the equator of the Bloch sphere. We perform a complete and comprehensive analysis of the optimal schemes based on local measurements, and give results (optimal measurements, maximum fidelity, etc.) for arbitrary N, not necessarily large, within the Bayesian framework. We also make a comparative analysis of the asymptotic limit of these results with those derived from a (pointwise) Cramer-Rao type of approach. We give explicit schemes based on local measurements and no classical communication that saturate the fidelity bounds of the most general collective schemes.

  18. Typicality of Pure States Randomly Sampled According to the Gaussian Adjusted Projected Measure

    NASA Astrophysics Data System (ADS)

    Reimann, Peter

    2008-09-01

    Consider a mixed quantum mechanical state, describing a statistical ensemble in terms of an arbitrary density operator ρ of low purity, tr ρ 2 ≪1, and yielding the ensemble averaged expectation value tr ( ρ A) for any observable A. Assuming that the given statistical ensemble ρ is generated by randomly sampling pure states | ψ> according to the corresponding so-called Gaussian adjusted projected measure (Goldstein et al. in J. Stat. Phys. 125:1197, 2006), the expectation value < ψ| A| ψ> is shown to be extremely close to the ensemble average tr ( ρ A) for the overwhelming majority of pure states | ψ> and any experimentally realistic observable A. In particular, such a `typicality' property holds whenever the Hilbert space ℋ of the system contains a high dimensional subspace ℋ+⊂ℋ with the property that all | ψ>∈ℋ+ are realized with equal probability and all other | ψ>∈ℋ are excluded.

  19. Manipulating topological states by imprinting non-collinear spin textures

    DOE PAGES

    Streubel, Robert; Han, Luyang; Im, Mi -Young; ...

    2015-03-05

    Topological magnetic states, such as chiral skyrmions, are of great scientific interest and show huge potential for novel spintronics applications, provided their topological charges can be fully controlled. So far skyrmionic textures have been observed in noncentrosymmetric crystalline materials with low symmetry and at low temperatures. We propose theoretically and demonstrate experimentally the design of spin textures with topological charge densities that can be tailored at ambient temperatures. Tuning the interlayer coupling in vertically stacked nanopatterned magnetic heterostructures, such as a model system of a Co/Pd multilayer coupled to Permalloy, the in-plane non-collinear spin texture of one layer can bemore » imprinted into the out-of-plane magnetised material. We observe distinct spin textures, e.g. vortices, magnetic swirls with tunable opening angle, donut states and skyrmion core configurations. We show that applying a small magnetic field, a reliable switching between topologically distinct textures can be achieved at remanence« less

  20. Manipulating topological states by imprinting non-collinear spin textures

    SciTech Connect

    Streubel, Robert; Han, Luyang; Im, Mi -Young; Kronast, Florian; Rößler, Ulrich K.; Radu, Florin; Abrudan, Radu; Schmidt, Oliver G.; Fischer, Peter; Makarov, Denys

    2015-03-05

    Topological magnetic states, such as chiral skyrmions, are of great scientific interest and show huge potential for novel spintronics applications, provided their topological charges can be fully controlled. So far skyrmionic textures have been observed in noncentrosymmetric crystalline materials with low symmetry and at low temperatures. We propose theoretically and demonstrate experimentally the design of spin textures with topological charge densities that can be tailored at ambient temperatures. Tuning the interlayer coupling in vertically stacked nanopatterned magnetic heterostructures, such as a model system of a Co/Pd multilayer coupled to Permalloy, the in-plane non-collinear spin texture of one layer can be imprinted into the out-of-plane magnetised material. We observe distinct spin textures, e.g. vortices, magnetic swirls with tunable opening angle, donut states and skyrmion core configurations. We show that applying a small magnetic field, a reliable switching between topologically distinct textures can be achieved at remanence

  1. Hydrogen bond-promoted metallic state in a purely organic single-component conductor under pressure.

    PubMed

    Isono, Takayuki; Kamo, Hiromichi; Ueda, Akira; Takahashi, Kazuyuki; Nakao, Akiko; Kumai, Reiji; Nakao, Hironori; Kobayashi, Kensuke; Murakami, Youichi; Mori, Hatsumi

    2013-01-01

    Purely organic materials are generally insulating. Some charge-carrier generation, however, can provide them with electrical conductivity. In multi-component organic systems, carrier generation by intermolecular charge transfer has given many molecular metals. By contrast, in purely organic single-component systems, metallic states have rarely been realized although some neutral-radical semiconductors have been reported. Here we uncover a new type of purely organic single-component molecular conductor by utilizing strong hydrogen-bonding interactions between tetrathiafulvalene-based electron-donor molecules. These conductors are composed of highly symmetric molecular units constructed by the strong intra-unit hydrogen bond. Moreover, we demonstrate that, in this system, charge carriers are produced by the partial oxidation of the donor molecules and delocalized through the formation of the symmetric intra-unit hydrogen bonds. As a result, our conductors show the highest room-temperature electrical conductivity and the metallic state under the lowest physical pressure among the purely organic single-component systems, to our knowledge.

  2. ``Spectral implementation'' for creating a labeled pseudo-pure state and the Bernstein-Vazirani algorithm in a four-qubit nuclear magnetic resonance quantum processor

    NASA Astrophysics Data System (ADS)

    Peng, Xinhua; Zhu, Xiwen; Fang, Ximing; Feng, Mang; Liu, Maili; Gao, Kelin

    2004-02-01

    A quantum circuit is introduced to describe the preparation of a labeled pseudo-pure state by multiplet-component excitation scheme which has been experimentally implemented on a 4-qubit nuclear magnetic resonance quantum processor. Meanwhile, we theoretically analyze and numerically investigate the low-power selective single-pulse implementation of a controlled-rotation gate, which manifests its validity in our experiment. Based on the labeled pseudo-pure state prepared, a 3-qubit Bernstein-Vazirani algorithm has been experimentally demonstrated by spectral implementation. The "answers" of the computations are identified from the split peak positions in the spectra of the observer spin, which are equivalent to projective measurements required by the algorithms.

  3. Spin-wave excitations in the spin-density wave state of doped iron pnictides.

    PubMed

    Singh, Dheeraj Kumar

    2017-10-18

    We investigate spin-wave excitations in the spin-density wave state of doped iron pnictides within a five-orbital model. We find that the excitations along ([Formula: see text])  →  ([Formula: see text]) are very sensitive to dopings whereas they do not exhibit a similar sensitivity along ([Formula: see text])  →  ([Formula: see text]). Secondly, the ellipticity of the elliptical ring-like excitations around ([Formula: see text]) is also very much dependent on doping. Thirdly, the spin-wave spectral weight shifts towards the low-energy region as it moves away from zero doping. We find several features to be in qualitative agreement with the inelastic neutron-scattering measurements for the doped pnictides.

  4. Relation Between Stereographic Projection and Concurrence Measure in Bipartite Pure States

    NASA Astrophysics Data System (ADS)

    Najarbashi, G.; Seifi, B.

    2016-10-01

    One-qubit pure states, living on the surface of Bloch sphere, can be mapped onto the usual complex plane by using stereographic projection. In this paper, after reviewing the entanglement of two-qubit pure state, it is shown that the quaternionic stereographic projection is related to concurrence measure. This is due to the fact that every two-qubit state, in ordinary complex field, corresponds to the one-qubit state in quaternionic skew field, called quaterbit. Like the one-qubit states in complex field, the stereographic projection maps every quaterbit onto a quaternion number whose complex and quaternionic parts are related to Schmidt and concurrence terms respectively. Rather, the same relation is established for three-qubit state under octonionic stereographic projection which means that if the state is bi-separable then, quaternionic and octonionic terms vanish. Finally, we generalize recent consequences to 2⊗ N and 4⊗ N dimensional Hilbert spaces ( N ≥ 2) and show that, after stereographic projection, the quaternionic and octonionic terms are entanglement sensitive. These trends are easily confirmed by direct computation for general multi-particle W- and GHZ-states.

  5. Terahertz electromagnons in spin-diluted cupric oxide: dynamics of twisted spin states

    NASA Astrophysics Data System (ADS)

    Lloyd-Hughes, James; Jones, Samuel; Wurz, Nicola; Failla, Michele; McConville, Chris; Prabhakaran, Dharmalingham

    2015-03-01

    Understanding the physics of magnetoelectric materials may lead to their application in actuators, sensors and solid state memories. Improper multiferroics also have novel quasiparticle excitations: electromagnons form when spin-waves become electric-dipole active. We investigated magnons, electromagnons and spin-lattice coupling in Cu(1-x)Zn(x)O (0spin-lattice coupling in Cu(1-x)Zn(x)O. While the phonon and magnon modes broaden and shift as a result of alloy-induced disorder, the electromagnon was found to be insensitive to Zn substitution and the induced disorder in the local spin structure. The results demonstrate that electromagnon excitations and dynamic magnetoelectric coupling can be maintained even in disordered spin systems, and at elevated temperatures.

  6. Enhanced Spin Squeezing in Atomic Ensembles via Control of the Internal Spin States

    NASA Astrophysics Data System (ADS)

    Shojaee, Ezad; Norris, Leigh; Baragiola, Ben; Montano, Enrique; Hemmer, Daniel; Jessen, Poul; Deutsch, Ivan

    2015-05-01

    Abstract: We study the process by which the collective spin squeezing of an ensemble of Cesium atoms is enhanced by control of the internal spin state of the atoms. By increasing the initial atomic projection noise, one can enhance the Faraday interaction that entangles the atoms with a probe. The light acts as a quantum bus for creating atom-atom entanglement via measurement backaction. Further control can be used to transfer this entanglement to metrologically useful squeezing. We numerically simulate this protocol by a stochastic master equation, including QND measurement and optical pumping, which accounts for decoherence and transfer of coherences between magnetic sub-levels. We study the tradeoff between the enhanced entangling interaction and increased rates of decoherence for different initial state preparations. Under realistic conditions, we find that we can achieve squeezing with a ``CAT-State'' superpostion |F = 4, Mz = 4> + |F, Mz = -4> of ~ 9.9 dB and for the spin coherent state |F = 4, Mx = 4> of ~ 7.5 dB. The increased entanglement enabled by the CAT state preparation is partially, but not completely reduced by the increased fragility to decoherence. National Science Foundation.

  7. Soft-x-ray-induced spin-state switching of an adsorbed Fe(II) spin-crossover complex

    NASA Astrophysics Data System (ADS)

    Kipgen, Lalminthang; Bernien, Matthias; Nickel, Fabian; Naggert, Holger; Britton, Andrew J.; Arruda, Lucas M.; Schierle, Enrico; Weschke, Eugen; Tuczek, Felix; Kuch, Wolfgang

    2017-10-01

    For probing the nature of spin-state switching in spin-crossover molecules adsorbed on surfaces, x-ray absorption spectroscopy has emerged as a powerful tool due to its high sensitivity and element selectivity in tracing even subtle electronic, magnetic, or chemical changes. However, the x-rays itself can induce a spin transition and might have unwanted influence while investigating the effect of other stimuli such as temperature or light, or of the surface, on the spin switching behaviour. Herein, we present the spin switching of an Fe(II) complex adsorbed on a highly oriented pyrolytic graphite surface with particular emphasis on the x-ray-induced switching. For a submonolayer coverage, the complex undergoes a complete and reversible temperature- and light-induced spin transition. The spin states are switched both ways by x-rays at 5 K, i.e. from the high-spin state to the low-spin state or vice versa, depending on the relative amount of each species. Furthermore, we quantify the fraction of molecules undergoing soft x-ray-induced photochemistry, a process which results in an irreversible low-spin state component, for a particular exposure time. This can be greatly suppressed by reducing the beam intensity.

  8. Soft-x-ray-induced spin-state switching of an adsorbed Fe(II) spin-crossover complex.

    PubMed

    Kipgen, Lalminthang; Bernien, Matthias; Nickel, Fabian; Naggert, Holger; Britton, Andrew J; Arruda, Lucas M; Schierle, Enrico; Weschke, Eugen; Tuczek, Felix; Kuch, Wolfgang

    2017-10-04

    For probing the nature of spin-state switching in spin-crossover molecules adsorbed on surfaces, x-ray absorption spectroscopy has emerged as a powerful tool due to its high sensitivity and element selectivity in tracing even subtle electronic, magnetic, or chemical changes. However, the x-rays itself can induce a spin transition and might have unwanted influence while investigating the effect of other stimuli such as temperature or light, or of the surface, on the spin switching behaviour. Herein, we present the spin switching of an Fe(II) complex adsorbed on a highly oriented pyrolytic graphite surface with particular emphasis on the x-ray-induced switching. For a submonolayer coverage, the complex undergoes a complete and reversible temperature- and light-induced spin transition. The spin states are switched both ways by x-rays at 5 K, i.e. from the high-spin state to the low-spin state or vice versa, depending on the relative amount of each species. Furthermore, we quantify the fraction of molecules undergoing soft x-ray-induced photochemistry, a process which results in an irreversible low-spin state component, for a particular exposure time. This can be greatly suppressed by reducing the beam intensity.

  9. Coherent control over three-dimensional spin polarization for the spin-orbit coupled surface state of Bi2Se3

    NASA Astrophysics Data System (ADS)

    Kuroda, Kenta; Yaji, Koichiro; Nakayama, M.; Harasawa, A.; Ishida, Y.; Watanabe, S.; Chen, C.-T.; Kondo, T.; Komori, F.; Shin, S.

    2016-10-01

    Interference of spin-up and spin-down eigenstates depicts spin rotation of electrons, which is a fundamental concept of quantum mechanics and presents technological challenges for the electrical spin manipulation. Here, we visualize this coherent spin physics through laser spin- and angle-resolved photoemission spectroscopy on a spin-orbital entangled surface state of a topological insulator. It is revealed that the linearly polarized laser can simultaneously excite spin-up and spin-down states, and these quantum-spin bases are coherently superposed in photoelectron states. The superposition and the resulting spin rotation is manipulated by the direction of the laser field. Moreover, the full observation of the spin rotation displays the phase of the quantum states. This presents a new facet of laser-photoemission technique for investigation of quantum-spin physics, opening new possibilities in the field of quantum spintronic applications.

  10. LABS problem and ground state spin glasses system

    NASA Astrophysics Data System (ADS)

    Leukhin, A. N.; Bezrodnyi, V. I.; Kozlova, Yu. A.

    2016-12-01

    In our work we demonstrate the new results of an exhaustive search for optimal binary sequences with minimum peak sidelobe (MPS) up to length N=85. The design problem for law autocorrelation binary sequences (LABS) is a notoriously difficult computational problem which is numbered as the problem number 005 in CSPLib. In statistical physics LABS problem can be interrepted as the energy of N iteracting Ising spins. This is a Bernasconi model. Due to this connection to physics we refer a binary sequence as one-dimensional spin lattice. At this assumption optimal binary sequences by merit factor (MF) criteria are the ground-state spin system without disorder which exhibits a glassy regime.

  11. Typicality in spin-network states of quantum geometry

    NASA Astrophysics Data System (ADS)

    Anza, Fabio; Chirco, Goffredo

    2016-10-01

    In this work, we extend the so-called typicality approach, originally formulated in statistical mechanics contexts, to S U (2 ) -invariant spin-network states. Our results do not depend on the physical interpretation of the spin network; however, they are mainly motivated by the fact that spin-network states can describe states of quantum geometry, providing a gauge-invariant basis for the kinematical Hilbert space of several background-independent approaches to quantum gravity. The first result is, by itself, the existence of a regime in which we show the emergence of a typical state. We interpret this as the proof that in that regime there are certain (local) properties of quantum geometry which are "universal." Such a set of properties is heralded by the typical state, of which we give the explicit form. This is our second result. In the end, we study some interesting properties of the typical state, proving that the area law for the entropy of a surface must be satisfied at the local level, up to logarithmic corrections which we are able to bound.

  12. Entangled states of spin and clock oscillators

    NASA Astrophysics Data System (ADS)

    Polzik, Eugene

    2016-05-01

    Measurements of one quadrature of an oscillator with precision beyond its vacuum state uncertainty have occupied a central place in quantum physics for decades. We have recently reported the first experimental implementation of such measurement with a magnetic oscillator. However, a much more intriguing goal is to trace an oscillator trajectory with the precision beyond the vacuum state uncertainty in both position and momentum, a feat naively assumed not possible due to the Heisenberg uncertainty principle. We have demonstrated that such measurement is possible if the oscillator is entangled with a quantum reference oscillator with an effective negative mass. The key element is the cancellation of the back action of the measurement on the composite system of two oscillators. Applications include measurements of e.-m. fields, accelleration, force and time with practically unlimited accuracy. In a more general sense, this approach leads to trajectories without quantum uncertainties and to achieving new fundamental bounds on the measurement precision.

  13. Direct measurement of the Concurrence of spin-entangled states in a cavity-quantum dot system

    NASA Astrophysics Data System (ADS)

    Dong, Ping; Liu, Jun; Zhang, Li-Hua; Cao, Zhuo-Liang

    2016-08-01

    A scheme for implementing the direct measurement of Concurrence is given in a cavity-quantum dot system. The scenario not only can directly measure the Concurrence of two-spin pure entangled state, but also suitable for the case of mixed state. More importantly, all of the operations are of geometric nature, which depend on the cavity-state-free evolution and can be robust against random operation errors. Our scheme provided an alternative method for directly measuring the degree of entanglement in solid-state system.

  14. Measurements of the spin states of Europa and Ganymede

    NASA Astrophysics Data System (ADS)

    Margot, Jean-Luc; Padovan, S.; Campbell, D.; Peale, S.; Ghigo, F.

    2013-10-01

    Measuring the spin states of the Galilean satellites holds the key to fundamental interior and surface properties. First, the spin state can reveal the presence of a subsurface ocean: a decoupling between the icy shell and the interior results in a different spin signature than that of a solid body. Second, the value of the obliquity combined with the known gravitational harmonics can provide a direct measurement of the polar moment of inertia, a crucial constraint on interior models. Finally, the obliquity may explain remarkable surface features, such as the distribution and shape of cycloids on Europa, and the direction of strike-slip faults. Here we present the first direct observations of the spin axis orientations of Europa and Ganymede. We use the same Earth-based radar technique that provided measurements of Mercury's obliquity at the sub-arcminute level, observational evidence that the core is molten, and core size estimates [1,2]. The measurements make simultaneous use of the Goldstone Solar System Radar and the Green Bank Telescope located ~3200 km away. It is the correlation of radar echoes received at these two stations that yields superb leverage on the spin state of the illuminated body. Because the Galilean satellites are further away than Mercury, and because they spin faster than Mercury, the signal-to-noise ratio of the observations is reduced by a factor of ~3000. Nevertheless, the telltale correlations are clearly detected in our data. Using measurements at 13 epochs in 2011 and 4 epochs in 2012, we are able to pinpoint Europa's spin axis orientation with a precision of ~0.1 deg, and our result is inconsistent with theoretical or model-based estimates [3,4,5]. For Ganymede, we secured measurements at 3 epochs in 2011 and 2 epochs in 2012, and the larger signal-to-noise ratio results in a comparable precision for the spin axis orientation. References [1] J. L. Margot et al. Science, 316:710, 2007. [2] J. L. Margot et al. JGR (Planets), 117(E16

  15. High-spin states and band terminations in 49V

    NASA Astrophysics Data System (ADS)

    Rodrigues, D.; Hojman, D.; Lenzi, S. M.; Cardona, M. A.; Farnea, E.; Axiotis, M.; Beck, C.; Bednarczyk, P.; Bizzetti, P. G.; Bizzetti-Sona, A. M.; Della Vedova, F.; Grebosz, J.; Haas, F.; Kmiecik, M.; Maj, A.; Meczyński, W.; Napoli, D. R.; Nespolo, M.; Papka, P.; Zafra, A. Sánchez i.; Styczen, J.; Thummerer, S.; Ziebliński, M.

    2015-08-01

    High-spin states in 49V have been studied through the 28Si(28Si,α 3 p ) reaction using the EUROBALL γ -ray detector array. The 49V level scheme has been extended up to 13.1 MeV including 21 new states. Both negative and positive parity states have been interpreted in the framework of the shell model. The 27 /2- and the 31/2 + band-termination states have been observed in agreement with theoretical predictions.

  16. Direct measurement of concurrence for atomic two-qubit pure states

    SciTech Connect

    Romero, G.; Lopez, C. E.; Lastra, F.; Retamal, J. C.; Solano, E.

    2007-03-15

    We propose a general scheme to measure the concurrence of an arbitrary two-qubit pure state in atomic systems. The protocol is based on one- and two-qubit operations acting on two available copies of the bipartite system, and followed by a global qubit readout. We show that it is possible to encode the concurrence in the probability of finding all atomic qubits in the ground state. Two possible scenarios are considered: atoms crossing three-dimensional microwave cavities and trapped ion systems.

  17. Fractional charge and spin states in topological insulator constrictions

    NASA Astrophysics Data System (ADS)

    Klinovaja, Jelena; Loss, Daniel

    2015-09-01

    We theoretically investigate the properties of two-dimensional topological insulator constrictions both in the integer and fractional regimes. In the presence of a perpendicular magnetic field, the constriction functions as a spin filter with near-perfect efficiency and can be switched by electric fields only. Domain walls between different topological phases can be created in the constriction as an interface between tunneling, magnetic fields, charge density wave, or electron-electron interaction dominated regions. These domain walls host non-Abelian bound states with fractional charge and spin and result in degenerate ground states with parafermions. If a proximity gap is induced bound states give rise to an exotic Josephson current with 8 π periodicity.

  18. Topological Phases in Graphene Nanoribbons: Junction States, Spin Centers, and Quantum Spin Chains

    NASA Astrophysics Data System (ADS)

    Cao, Ting; Zhao, Fangzhou; Louie, Steven G.

    2017-08-01

    We show that semiconducting graphene nanoribbons (GNRs) of different width, edge, and end termination (synthesizable from molecular precursors with atomic precision) belong to different electronic topological classes. The topological phase of GNRs is protected by spatial symmetries and dictated by the terminating unit cell. We have derived explicit formulas for their topological invariants and shown that localized junction states developed between two GNRs of distinct topology may be tuned by lateral junction geometry. The topology of a GNR can be further modified by dopants, such as a periodic array of boron atoms. In a superlattice consisting of segments of doped and pristine GNRs, the junction states are stable spin centers, forming a Heisenberg antiferromagnetic spin 1 /2 chain with tunable exchange interaction. The discoveries here not only are of scientific interest for studies of quasi-one-dimensional systems, but also open a new path for design principles of future GNR-based devices through their topological characters.

  19. Emergence of equilibrium thermodynamic properties in quantum pure states. I. Theory

    SciTech Connect

    Fresch, Barbara; Moro, Giorgio J.

    2010-07-21

    Investigation on foundational aspects of quantum statistical mechanics recently entered a renaissance period due to novel intuitions from quantum information theory and to increasing attention on the dynamical aspects of single quantum systems. In the present contribution a simple but effective theoretical framework is introduced to clarify the connections between a purely mechanical description and the thermodynamic characterization of the equilibrium state of an isolated quantum system. A salient feature of our approach is the very transparent distinction between the statistical aspects and the dynamical aspects in the description of isolated quantum systems. Like in the classical statistical mechanics, the equilibrium distribution of any property is identified on the basis of the time evolution of the considered system. As a consequence equilibrium properties of quantum system appear to depend on the details of the initial state due to the abundance of constants of the motion in the Schroedinger dynamics. On the other hand the study of the probability distributions of some functions, such as the entropy or the equilibrium state of a subsystem, in statistical ensembles of pure states reveals the crucial role of typicality as the bridge between macroscopic thermodynamics and microscopic quantum dynamics. We shall consider two particular ensembles: the random pure state ensemble and the fixed expectation energy ensemble. The relation between the introduced ensembles, the properties of a given isolated system, and the standard quantum statistical description are discussed throughout the presentation. Finally we point out the conditions which should be satisfied by an ensemble in order to get meaningful thermodynamical characterization of an isolated quantum system.

  20. Static spin susceptibility in magnetically ordered states

    NASA Astrophysics Data System (ADS)

    Kuboki, Kazuhiro; Yamase, Hiroyuki

    2017-08-01

    We report that special care is needed when longitudinal magnetic susceptibility is computed in a magnetically ordered phase, especially in metals. We demonstrate this by studying static susceptibility in both a ferromagnetic and an antiferromagnetic state in the random phase approximation to the two-dimensional Hubbard model on a square lattice. In contrast to the case in the disordered phase, a first derivative of the chemical potential (or the density) with respect to a magnetic field does not vanish in a magnetically ordered phase when the field is applied parallel to the magnetic moment. This effect is crucial and should be included when computing magnetic susceptibility in the ordered phase, otherwise an unphysical result would be obtained. In addition, consequently the magnetic susceptibility becomes different when computed at a fixed density and a fixed chemical potential in the ordered phase. In particular, we cannot employ magnetic susceptibility at a fixed chemical potential to describe a system with a fixed density even if the chemical potential is tuned to reproduce the correct density.

  1. Entanglement in bipartite pure states of an interacting boson gas obtained by local projective measurements

    SciTech Connect

    Paraan, Francis N. C.; Korepin, Vladimir E.; Molina-Vilaplana, Javier; Bose, Sougato

    2011-09-15

    We quantify the extractable entanglement of excited states of a Lieb-Liniger gas that are obtained from coarse-grained measurements on the ground state in which the boson number in one of two complementary contiguous partitions of the gas is determined. Numerically exact results obtained from the coordinate Bethe ansatz show that the von Neumann entropy of the resulting bipartite pure state increases monotonically with the strength of repulsive interactions and saturates to the impenetrable-boson limiting value. We also present evidence indicating that the largest amount of entanglement can be extracted from the most probable projected state having half the number of bosons in a given partition. Our study points to a fundamental difference between the nature of the entanglement in free-bosonic and free-fermionic systems, with the entanglement in the former being zero after projection, while that in the latter (corresponding to the impenetrable-boson limit) being nonzero.

  2. An equation of state for purely kinetic k-essence inspired by cosmic topological defects

    NASA Astrophysics Data System (ADS)

    Cordero, Rubén; González, Eduardo L.; Queijeiro, Alfonso

    2017-06-01

    We investigate the physical properties of a purely kinetic k-essence model with an equation of state motivated in superconducting membranes. We compute the equation of state parameter w and discuss its physical evolution via a nonlinear equation of state. Using the adiabatic speed of sound and energy density, we restrict the range of parameters of the model in order to have an acceptable physical behavior. We study the evolution of the scale factor and address the question of the possible existence of finite-time future singularities. Furthermore, we analyze the evolution of the luminosity distance dL with redshift z by comparing (normalizing) it with the Λ CDM model. Since the equation of state parameter is z-dependent the evolution of the luminosity distance is also analyzed using the Alcock-Paczyński test.

  3. Y{sub 3}Fe{sub 5}O{sub 12} spin pumping for quantitative understanding of pure spin transport and spin Hall effect in a broad range of materials (invited)

    SciTech Connect

    Du, Chunhui; Wang, Hailong; Hammel, P. Chris; Yang, Fengyuan

    2015-05-07

    Using Y{sub 3}Fe{sub 5}O{sub 12} (YIG) thin films grown by our sputtering technique, we study dynamic spin transport in nonmagnetic, ferromagnetic, and antiferromagnetic (AF) materials by ferromagnetic resonance spin pumping. From both inverse spin Hall effect and damping enhancement, we determine the spin mixing conductance and spin Hall angle in many metals. Surprisingly, we observe robust spin conduction in AF insulators excited by an adjacent YIG at resonance. This demonstrates that YIG spin pumping is a powerful and versatile tool for understanding spin Hall physics, spin-orbit coupling, and magnetization dynamics in a broad range of materials.

  4. Ground-state valency and spin configuration of the nickelates.

    NASA Astrophysics Data System (ADS)

    Petit, Leon; Stocks, George M.; Egami, Takeshi; Szotek, Zdzislawa; Temmerman, Walter M.

    2006-03-01

    The ab initio self-interaction-corrected local-spin-density approximation is used to study the electronic structure of both stoichiometric and non-stoichiometric nickelates. From total energy considerations it emerges that, in their ground-state, both LiNiO2, and NaNiO2 are insulators, with the Ni ion in the Ni^3+ low spin state (t2g^6eg^1) configuration. We find that the substitution of Li/Na atoms by divalent impurities, drives an equivalent number of Ni ions in the NiO2 layers from the JT-active trivalent low-spin state to the divalent JT-inactive state. We propose that an experimental study on MgxNa1-xNiO2 might clarify the role of Ni^2+ impurities with respect to the vanishing of long range orbital ordering in Li1-xNi1+xO2. (Work sponsored by the Laboratory Directed Research and Development Program (LDRD) program of ORNL (LP, GMS, TE), and by the DOE-OS through the Offices of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering (LP, GMS, TE). Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the Department of Energy under Contract No. DE-AC05-00OR22725.)

  5. Spin-flop states in a synthetic antiferromagnet and variations of unidirectional anisotropy in FeMn-based spin valves

    NASA Astrophysics Data System (ADS)

    Milyaev, M. A.; Naumova, L. I.; Chernyshova, T. A.; Proglyado, V. V.; Kulesh, N. A.; Patrakov, E. I.; Kamenskii, I. Yu.; Ustinov, V. V.

    2016-12-01

    Spin valves with a synthetic antiferromagnet have been prepared by magnetron sputtering. Regularities of the formation of single- and two-phase spin-flop states in the synthetic antiferromagnet have been studied using magnetoresistance measurements and imaging the magnetic structure. A thermomagnetic treatment of spin valve in a field that corresponds to the single-phase spin-flop state of synthetic antiferromagnet was shown to allow us to obtain a magnetically sensitive material characterized by hysteresis-free field dependence of the magnetoresistance.

  6. Four and Five-body non-local correlations in pure and mixed states

    NASA Astrophysics Data System (ADS)

    Sharma, Santosh Shelly; Sharma, Naresh Kumar

    2014-03-01

    In our earlier works, quantifiers of four and three-body correlations based on four qubit invariants had been constructed for pure states. The principal construction tools, local unitary invariance and notion of negativity fonts, make it possible to outline the process of selective construction of meaningful invariants that quanify N and N - 1 qubit correlations. It is found that, in general, starting from degree k invariants relevant to detection and quantifcation of specific type of non-local quantum correlations in (N - 1) (N > 2) qubit system, one can construct degree k coefficients of an N-qubit bilinear form. When k =2 N - 2 (N > 2), one of the invariants of degree 2 N - 1 quantifies N-body non-local correlations The process is recursive. While for few body systems it yields analytical expressions in terms of functions of state coefficients, for larger systems it can be the guiding principle to numerical caculations of invariants. To illustrate the process, an expression for a five qubit correlation quantifier for pure states is constructed. In addition, the extension to specific rank two mixed states through convex-roof extension is investigated. We gratefully acknowledge Financial support from CNPq Brazil and Fundacao Araucaria PR Brazil.

  7. Bound states of spinning black holes in five dimensions

    NASA Astrophysics Data System (ADS)

    Crichigno, P. Marcos; Porri, Flavio; Vandoren, Stefan

    2017-05-01

    We find and study supergravity BPS bound states of five-dimensional spinning black holes in asymptotically flat spacetime. These solutions follow from multi-string solutions in six-dimensional minimal supergravity and can be uplifted to F-theory or M-theory. We analyze the regularity conditions and work out the example of a bound state of two black holes in detail. The bound state is supported by fluxes through nontrivial topologies exterior to the horizons and KK momentum. Furthermore, we determine the entropy and compare with other macroscopic BPS solutions.

  8. Spins of Andreev states in double quantum dots

    NASA Astrophysics Data System (ADS)

    Su, Zhaoen; Chen, Jun; Yu, Peng; Hocervar, Moira; Plissard, Sebastien; Car, Diana; Tacla, Alexandre; Daley, Andrew; Pekker, David; Bakkers, Erik; Frolov, Sergey

    Andreev (or Shiba) states in coupled double quantum dots is an open field. Here we demonstrate the realization of Andreev states in double quantum dots in an InSb nanowire coupled to two NbTiN superconductors. The magnetic field dependence of the Andreev states has been explored to resolve the spins in different double dot configurations. The experiment helps to understand the interplay between pair correlation, exchange energy and charging energy with a well-controlled system. It also opens the possibility to implement Majorana modes in Kitaev chains made of such dots.

  9. Exotic Paired States with Anisotropic Spin-Dependent Fermi Surfaces

    SciTech Connect

    Feiguin, Adrian E.; Fisher, Matthew P. A.

    2009-07-10

    We propose a model for realizing exotic paired states in cold Fermi gases by using a spin-dependent optical lattice to engineer mismatched Fermi surfaces for each hyperfine species. The BCS phase diagram shows a stable paired superfluid state with coexisting pockets of momentum space with gapless unpaired carriers, similar to the Sarma state in polarized mixtures, but in our case the system is unpolarized. We propose the possible existence of an exotic 'Cooper-pair Bose-metal' phase, which has a gap for single fermion excitations but gapless and uncondensed 'Cooper-pair' excitations residing on a 'Bose surface' in momentum space.

  10. Physics and application of persistent spin helix state in semiconductor heterostructures

    NASA Astrophysics Data System (ADS)

    Kohda, Makoto; Salis, Gian

    2017-07-01

    In order to utilize the spin degree of freedom in semiconductors, control of spin states and transfer of the spin information are fundamental requirements for future spintronic devices and quantum computing. Spin orbit (SO) interaction generates an effective magnetic field for moving electrons and enables spin generation, spin manipulation and spin detection without using external magnetic field and magnetic materials. However, spin relaxation also takes place due to a momentum dependent SO-induced effective magnetic field. As a result, SO interaction is considered to be a double-edged sword facilitating spin control but preventing spin transport over long distances. The persistent spin helix (PSH) state solves this problem since uniaxial alignment of the SO field with SU(2) symmetry enables the suppression of spin relaxation while spin precession can still be controlled. Consequently, understanding the PSH becomes an important step towards future spintronic technologies for classical and quantum applications. Here, we review recent progress of PSH in semiconductor heterostructures and its device application. Fundamental physics of SO interaction and the conditions of a PSH state in semiconductor heterostructures are discussed. We introduce experimental techniques to observe a PSH and explain both optical and electrical measurements for detecting a long spin relaxation time and the formation of a helical spin texture. After emphasizing the bulk Dresselhaus SO coefficient γ, the application of PSH states for spin transistors and logic circuits are discussed.

  11. Exact spin-cluster ground states in a mixed diamond chain

    NASA Astrophysics Data System (ADS)

    Takano, Ken'Ichi; Suzuki, Hidenori; Hida, Kazuo

    2009-09-01

    The mixed diamond chain is a frustrated Heisenberg chain composed of successive diamond-shaped units with two kinds of spins of magnitudes S and S/2 ( S : integer). Ratio λ of two exchange parameters controls the strength of frustration. With varying λ , the Haldane state and several spin-cluster states appear as the ground state. A spin-cluster state is a tensor product of exact local eigenstates of cluster spins. We prove that a spin-cluster state is the ground state in a finite interval of λ . For S=1 , we numerically determine the total phase diagram consisting of five phases.

  12. Minimum energy trap states of dual-spin spacecraft

    NASA Technical Reports Server (NTRS)

    Hollars, M. G.

    1980-01-01

    The general solution to the bearing axis motor torque required to escape a minimum energy trap state is presented for oblate dual-spin spacecraft. A simplified, reduced order analysis of the bearing torque is then obtained for the case of small static imbalances, dynamic imbalances, and asymmetries on the rotor and the stator. This analysis is extended to include large asymmetry on one of the bodies. The results are applied to the design of the Galileo spacecraft.

  13. Observation of Excited State Spin Ordering under Pulsed Magnetic Field

    NASA Astrophysics Data System (ADS)

    Amaya, Kiichi; Karaki, Yoshitomo; Yamada, Norikatsu; Haseda, Taiichiro

    1981-10-01

    Spin ordering among excited levels in NaNi Acac3\\cdotbenzene is observed in the course of pulsed adiabatic magnetization with sweep rate of 105 T/sec. For initial temperatures below 1 K, dM/dt signals give the characteristic double peaks around the field of 2.11 T where the excited singlet and the upper state of the ground doublet crosses.

  14. Lifetime measurement of high spin states in (75) Kr

    SciTech Connect

    Sheikh, Javid; Trivedi, T.; Maurya, K.; Mehrotra, I.; Palit, R.; Naik, Z.; Jain, H. C.; Negi, D.; Mahanto, G.; Kumar, R.; Singh, R.P.; Muralithar, S.; Pancholi, S.C.; Bhowmik, R.K.; Yang, Y-C; Sun, Y.; Dahl, A.; Raju, M.K.; Appannababu, S.; Kumar, S.; Choudhury, D.; Jain, A. K.

    2010-01-01

    The lifetimes of high spin states of {sup 75}Kr have been determined via {sup 50}Cr ({sup 28}Si, 2pn) {sup 75}Kr reaction in positive parity band using the Doppler-shift attenuation method. The transition quadrupole moments Q deduced from lifetime measurements have been compared with {sup 75}Br. Experimental results obtained from lifetime measurement are interpreted in the framework of projected shell model.

  15. Lifetimes of high-spin states in {sup 162}Yb

    SciTech Connect

    Carpenter, M.P.; Janssens, R.V.F.; Henry, R.G.

    1995-08-01

    A measurement on lifetimes of high-spin states in the yrast and near-yrast rotational bands in {sup 162}Yb was carried out at ATLAS in order to determine the evolution of collectivity as a function of angular momentum using the {sup 126}Te({sup 40}Ar,4n){sup 162}Yb reaction at 170 MeV. Previous lifetime measurements in the {sup 164,166,168}Yb isotopes showed a dramatic decrease in the transition quadrupole moment Q{sub t} with increasing spin. It was suggested that this decrease in Q{sub t} is brought about by the rotationally-induced deoccupation of high-j configurations, mainly i{sub 13/2} neutrons. If this interpretation is correct, the heavier isotopes should have a larger decrease in Q{sub t} than the lighter mass nuclides due to the position of the Fermi surface in the i{sub 13/2} subshell. Indeed, {sup 160}Yb does not show a clear decrease in Q{sub t} at high spin. No high spin lifetime information exists for {sup 162}Yb, thus this experiment fills the gap of measured Q{sub t}`s in the light Yb series. The data is currently being analyzed.

  16. SPIN STATE AND MOMENT OF INERTIA CHARACTERIZATION OF 4179 TOUTATIS

    SciTech Connect

    Takahashi, Yu; Scheeres, D. J.; Busch, Michael W.

    2013-10-01

    The 4.5 km long near-Earth asteroid 4179 Toutatis has made close Earth flybys approximately every four years between 1992 and 2012, and has been observed with high-resolution radar imaging during each approach. Its most recent Earth flyby in 2012 December was observed extensively at the Goldstone and Very Large Array radar telescopes. In this paper, Toutatis' spin state dynamics are estimated from observations of five flybys between 1992 and 2008. Observations were used to fit Toutatis' spin state dynamics in a least-squares sense, with the solar and terrestrial tidal torques incorporated in the dynamical model. The estimated parameters are Toutatis' Euler angles, angular velocity, moments of inertia, and the center-of-mass-center-of-figure offset. The spin state dynamics as well as the uncertainties of the Euler angles and angular velocity of the converged solution are then propagated to 2012 December in order to compare the dynamical model to the most recent Toutatis observations. The same technique of rotational dynamics estimation can be applied to any other tumbling body, given sufficiently accurate observations.

  17. Spin State and Moment of Inertia Characterization of 4179 Toutatis

    NASA Astrophysics Data System (ADS)

    Takahashi, Yu; Busch, Michael W.; Scheeres, D. J.

    2013-10-01

    The 4.5 km long near-Earth asteroid 4179 Toutatis has made close Earth flybys approximately every four years between 1992 and 2012, and has been observed with high-resolution radar imaging during each approach. Its most recent Earth flyby in 2012 December was observed extensively at the Goldstone and Very Large Array radar telescopes. In this paper, Toutatis' spin state dynamics are estimated from observations of five flybys between 1992 and 2008. Observations were used to fit Toutatis' spin state dynamics in a least-squares sense, with the solar and terrestrial tidal torques incorporated in the dynamical model. The estimated parameters are Toutatis' Euler angles, angular velocity, moments of inertia, and the center-of-mass-center-of-figure offset. The spin state dynamics as well as the uncertainties of the Euler angles and angular velocity of the converged solution are then propagated to 2012 December in order to compare the dynamical model to the most recent Toutatis observations. The same technique of rotational dynamics estimation can be applied to any other tumbling body, given sufficiently accurate observations.

  18. π Spin Berry Phase in a Quantum-Spin-Hall-Insulator-Based Interferometer: Evidence for the Helical Spin Texture of the Edge States

    NASA Astrophysics Data System (ADS)

    Chen, Wei; Deng, Wei-Yin; Hou, Jing-Min; Shi, D. N.; Sheng, L.; Xing, D. Y.

    2016-08-01

    The quantum spin Hall insulator is characterized by helical edge states, with the spin polarization of the electron being locked to its direction of motion. Although the edge-state conduction has been observed, unambiguous evidence of the helical spin texture is still lacking. Here, we investigate the coherent edge-state transport in an interference loop pinched by two point contacts. Because of the helical character, the forward interedge scattering enforces a π spin rotation. Two successive processes can only produce a nontrivial 2 π or trivial 0 spin rotation, which can be controlled by the Rashba spin-orbit coupling. The nontrivial spin rotation results in a geometric π Berry phase, which can be detected by a π phase shift of the conductance oscillation relative to the trivial case. Our results provide smoking gun evidence for the helical spin texture of the edge states. Moreover, it also provides the opportunity to all electrically explore the trajectory-dependent spin Berry phase in condensed matter.

  19. π Spin Berry Phase in a Quantum-Spin-Hall-Insulator-Based Interferometer: Evidence for the Helical Spin Texture of the Edge States.

    PubMed

    Chen, Wei; Deng, Wei-Yin; Hou, Jing-Min; Shi, D N; Sheng, L; Xing, D Y

    2016-08-12

    The quantum spin Hall insulator is characterized by helical edge states, with the spin polarization of the electron being locked to its direction of motion. Although the edge-state conduction has been observed, unambiguous evidence of the helical spin texture is still lacking. Here, we investigate the coherent edge-state transport in an interference loop pinched by two point contacts. Because of the helical character, the forward interedge scattering enforces a π spin rotation. Two successive processes can only produce a nontrivial 2π or trivial 0 spin rotation, which can be controlled by the Rashba spin-orbit coupling. The nontrivial spin rotation results in a geometric π Berry phase, which can be detected by a π phase shift of the conductance oscillation relative to the trivial case. Our results provide smoking gun evidence for the helical spin texture of the edge states. Moreover, it also provides the opportunity to all electrically explore the trajectory-dependent spin Berry phase in condensed matter.

  20. Light-Induced Spin State Switching and Relaxation in Spin Pairs of Copper(II)-Nitroxide Based Molecular Magnets.

    PubMed

    Tumanov, Sergey V; Veber, Sergey L; Tolstikov, Svyatoslav E; Artiukhova, Natalia A; Romanenko, Galina V; Ovcharenko, Victor I; Fedin, Matvey V

    2017-10-02

    Similar to spin-crossover (SCO) compounds, spin states of copper(II)-nitroxide based molecular magnets can be switched by various external stimuli including temperature and light. Although photoswitching and reverse relaxation of nitroxide-copper(II)-nitroxide triads were investigated in some detail, similar study for copper(II)-nitroxide spin pairs was still missing. In this work we address photoswitching and relaxation phenomena in exchange-coupled spin pairs of this family of molecular magnets. Using electron paramagnetic resonance (EPR) spectroscopy with photoexcitation, we demonstrate that compared to triad-containing compounds the photoinduced weakly coupled spin (WS) states of copper(II)-nitroxide pairs are remarkably more stable at cryogenic temperatures and relax to the ground strongly coupled spin (SS) states on the scale of days. The structural changes between SS and WS states, e.g., differences in Cu-Onitroxide distances, are much more pronounced for spin pairs than for spin triads in most of the studied copper(II)-nitroxide based molecular magnets. This results in higher energy barrier between WS and SS states of spin pairs and governs higher stability of their photoinduced WS states. Therefore, the longer-lived photoinduced states in copper(II)-nitroxide molecular magnets should be searched within the compounds experiencing largest structural changes upon thermal spin transition. This advancement in understanding of LIESST-like phenomena in copper(II)-nitroxide molecular magnets allows us to propose them as interesting playgrounds for benchmarking the basic factors governing the stability of photoinduced states in other SCO and SCO-like photoswitchable systems.

  1. Photophysical processes of triplet states and radical ions in pure and molecularly doped polymers. Final report

    SciTech Connect

    Burkhart, R.D.

    1998-01-01

    Both the past and current objectives are to learn how to control the rate and direction of triplet exciton migration in both pure and molecularly doped polymer systems. Since triplet excimers are efficient traps for migrating excitons, a secondary objective has been to characterize these excimers with a view toward their use as rate modifiers or excited state quenchers. Further objectives included those stated above as past and current objectives but with an additional goal. The authors learned that fluid solutions of many of the nitrogen containing chromophores with which they work produce both radical cations and anions upon excimer laser excitation. They also learned that a phosphorus analogue behaves similarly. At this time the mechanism of charge generation in these systems is not well established but they do know that the electronically excited states and radical ions can potentially interconvert. They wanted to find out whether or not the pure or molecularly doped polymer systems could be used in a step-wise sequence involving light absorption followed by charge generation. All of their activities are oriented toward the potential end use of polymeric systems in the conversion of light energy to perform various types of useful work.

  2. Entanglement manipulation of multipartite pure states with finite rounds of classical communication

    NASA Astrophysics Data System (ADS)

    de Vicente, J. I.; Spee, C.; Sauerwein, D.; Kraus, B.

    2017-01-01

    We studied pure state transformations using local operations assisted by finitely many rounds of classical communication (LOCCIN) [C. Spee, J. I. de Vicente, D. Sauerwein, and B. Kraus [Phys. Rev. Lett. (to be published)], arXiv:1606.04418]. Here, we present the details of some of the proofs and generalize the construction of examples of state transformations via LOCCIN which require a probabilistic step. However, we also present explicit examples of SLOCC classes where any separable transformation can be realized by a protocol in which each step is deterministic (all-det-LOCCIN). Such transformations can be considered as natural generalizations of bipartite transformations. Furthermore, we provide examples of pure state transformations which are possible via separable transformations, but not via LOCCIN. We also analyze an interesting genuinely multipartite effect which we call locking or unlocking the power of other parties. This means that one party can prevent or enable the implementation of LOCC transformations by other parties. Moreover, we investigate the maximally entangled set restricted to LOCCIN and show how easily computable bounds on some entanglement measures can be derived by restricting to LOCCIN.

  3. Decoherence and thermalization of a pure quantum state in quantum field theory.

    PubMed

    Giraud, Alexandre; Serreau, Julien

    2010-06-11

    We study the real-time evolution of a self-interacting O(N) scalar field initially prepared in a pure, coherent quantum state. We present a complete solution of the nonequilibrium quantum dynamics from a 1/N expansion of the two-particle-irreducible effective action at next-to-leading order, which includes scattering and memory effects. We demonstrate that, restricting one's attention (or ability to measure) to a subset of the infinite hierarchy of correlation functions, one observes an effective loss of purity or coherence and, on longer time scales, thermalization. We point out that the physics of decoherence is well described by classical statistical field theory.

  4. Quantum pump in quantum spin Hall edge states

    NASA Astrophysics Data System (ADS)

    Cheng, Fang

    2016-09-01

    We present a theory for quantum pump in a quantum spin Hall bar with two quantum point contacts (QPCs). The pump currents can be generated by applying harmonically modulating gate voltages at QPCs. The phase difference between the gate voltages introduces an effective gauge field, which breaks the time-reversal symmetry and generates pump currents. The pump currents display very different pump frequency dependence for weak and strong e-e interaction. These unique properties are induced by the helical feature of the edge states, and therefore can be used to detect and control edge state transport.

  5. Interference of spin states in resonant photoemission induced by circularly polarized light from magnetized Gd

    SciTech Connect

    Mueller, N.; Khalil, T.; Pohl, M.; Uphues, T.; Heinzmann, U.; Polcik, M.; Rader, O.; Heigl, F.; Starke, K.; Fritzsche, S.; Kabachnik, N. M.

    2006-10-15

    We have observed the spin-state interference by measuring the photoelectron spin polarization in the resonant preedge 4d{yields}4f photoemission from magnetized Gd. The photoemission is induced by circularly polarized light which determines one preferential direction of electron spin orientation due to polarization transfer and spin-orbit interaction. Another direction perpendicular to the first one is determined by the target electron spin orientation connected with the target magnetization. We have measured the component of spin polarization perpendicular to those two directions which can only appear due to spin-state interference which implies coherence of the spin states produced by the two mechanisms of the photoelectron spin polarization.

  6. Quantifying entanglement of arbitrary-dimensional multipartite pure states in terms of the singular values of coefficient matrices

    NASA Astrophysics Data System (ADS)

    Li, Hui; Wang, Shuhao; Cui, Jianlian; Long, Guilu

    2013-04-01

    The entanglement quantification and classification of multipartite quantum states are two important research fields in quantum information. In this work, we study the entanglement of arbitrary-dimensional multipartite pure states by looking at the averaged partial entropies of various bipartite partitions of the system, namely, the so-called Manhattan distance (l1 norm) of averaged partial entropies (MAPE), and it is proved to be an entanglement measure for pure states. We connected the MAPE with the coefficient matrices, which are important tools in entanglement classification and reexpressed the MAPE for arbitrary-dimensional multipartite pure states by the nonzero singular values of the coefficient matrices. The entanglement properties of the n-qubit Dicke states, arbitrary-dimensional Greenberger-Horne-Zeilinger states, and D3n states are investigated in terms of the MAPE, and the relation between the rank of the coefficient matrix and the degree of entanglement is demonstrated for symmetric states by two examples.

  7. Minimum error discrimination for an ensemble of linearly independent pure states

    NASA Astrophysics Data System (ADS)

    Singal, Tanmay; Ghosh, Sibasish

    2016-04-01

    Inspired by the work done by Belavkin (1975 Stochastics 1 315) and independently by Mochon, (2006 Phys. Rev. A 73 032328), we formulate the problem of minimum error discrimination (MED) of any ensemble of n linearly independent pure states by stripping the problem of its rotational covariance and retaining only the rotationally invariant aspect of the problem. This is done by embedding the optimal conditions in a matrix equality as well as matrix inequality. Employing the implicit function theorem in these conditions we get a set of first-order coupled ordinary nonlinear differential equations which can be used to drag the solution from an initial point (where solution is known) to another point (whose solution is sought). This way of obtaining the solution can be done through a simple Taylor series expansion and analytic continuation when required. Thus, we complete the work done by Belavkin and Mochon by ultimately leading their theory to a solution for the MED problem of linearly independent pure state ensembles. We also compare the computational complexity of our technique with the barrier-type interior point method of SDP and show that our technique is computationally as efficient as (actually, a bit more than) the SDP algorithm, with the added advantage of being much simpler to implement.

  8. Floquet spin states in graphene under ac-driven spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    López, A.; Sun, Z. Z.; Schliemann, J.

    2012-05-01

    We study the role of periodically driven time-dependent Rashba spin-orbit coupling (RSOC) on a monolayer graphene sample. After recasting the originally 4×4 system of dynamical equations as two time-reversal related two-level problems, the quasienergy spectrum and the related dynamics are investigated via various techniques and approximations. In the static case, the system is gapped at the Dirac point. The rotating wave approximation (RWA) applied to the driven system unphysically preserves this feature, while the Magnus-Floquet approach as well as a numerically exact evaluation of the Floquet equation show that this gap is dynamically closed. In addition, a sizable oscillating pattern of the out-of-plane spin polarization is found in the driven case for states that are completely unpolarized in the static limit. Evaluation of the autocorrelation function shows that the original uniform interference pattern corresponding to time-independent RSOC gets distorted. The resulting structure can be qualitatively explained as a consequence of the transitions induced by the ac driving among the static eigenstates, i.e., these transitions modulate the relative phases that add up to give the quantum revivals of the autocorrelation function. Contrary to the static case, in the driven scenario, quantum revivals (suppressions) are correlated to spin-up (down) phases.

  9. Cox’s Chair Revisited: Can Spinning Alter Mood States?

    PubMed Central

    Winter, Lotta; Wollmer, M. Axel; Laurens, Jean; Straumann, Dominik; Kruger, Tillmann H. C.

    2013-01-01

    Although there is clinical and historical evidence for a vivid relation between the vestibular and emotional systems, the neuroscientific underpinnings are poorly understood. The “spin doctors” of the nineteenth century used spinning chairs (e.g., Cox’s chair) to treat conditions of mania or elevated arousal. On the basis of a recent study on a hexapod motion-simulator, in this prototypic investigation we explore the impact of yaw stimulation on a spinning chair on mood states. Using a controlled experimental stimulation paradigm on a unique 3-D-turntable at the University of Zurich we included 11 healthy subjects and assessed parameters of mood states and autonomic nervous system activity. The Multidimensional Mood State Questionnaire and Visual Analog Scales (VAS) were used to assess changes of mood in response to a 100 s yaw stimulation. In addition heart rate was continuously monitored during the experiment. Subjects indicated feeling less “good,” “relaxed,” “comfortable,” and “calm” and reported an increased alertness after vestibular stimulation. However, there were no objective adverse effects of the stimulation. Accordingly, heart rate did not significantly differ in response to the stimulation. This is the first study in a highly controlled setting using the historical approach of stimulating the vestibular system to impact mood states. It demonstrates a specific interaction between the vestibular system and mood states and thereby supports recent experimental findings with a different stimulation technique. These results may inspire future research on the clinical potential of this method. PMID:24133463

  10. Models of the spin state of the comet Halley nucleus

    NASA Technical Reports Server (NTRS)

    Julian, William H.

    1990-01-01

    Eight rotation precession models of the comet Halley nucleus have been proposed by eight authors. The eight models were evaluated in relation to the constraints imposed by: (1) the observed long axis directions at the Vega 1, Vega 2, and Giotto encounters; (2) the ground based emission periods harmonically related to 7.4 days; (3) the need for a two day spin period in the analysis of the jet morphology; (4) the Smith et al. constraint on the net long axis roll between Vega 2 and Giotto; (5) the resistance of the spin state of the nucleus to change due to the torque from the jets; and (6) the 7.4 day repetition of the spatial orientation of the nucleus. The eight constraints are briefly described.

  11. Retrieving the ground state of spin glasses using thermal noise: Performance of quantum annealing at finite temperatures.

    PubMed

    Nishimura, Kohji; Nishimori, Hidetoshi; Ochoa, Andrew J; Katzgraber, Helmut G

    2016-09-01

    We study the problem to infer the ground state of a spin-glass Hamiltonian using data from another Hamiltonian with interactions disturbed by noise from the original Hamiltonian, motivated by the ground-state inference in quantum annealing on a noisy device. It is shown that the average Hamming distance between the inferred spin configuration and the true ground state is minimized when the temperature of the noisy system is kept at a finite value, and not at zero temperature. We present a spin-glass generalization of a well-established result that the ground state of a purely ferromagnetic Hamiltonian is best inferred at a finite temperature in the sense of smallest Hamming distance when the original ferromagnetic interactions are disturbed by noise. We use the numerical transfer-matrix method to establish the existence of an optimal finite temperature in one- and two-dimensional systems. Our numerical results are supported by mean-field calculations, which give an explicit expression of the optimal temperature to infer the spin-glass ground state as a function of variances of the distributions of the original interactions and the noise. The mean-field prediction is in qualitative agreement with numerical data. Implications on postprocessing of quantum annealing on a noisy device are discussed.

  12. Retrieving the ground state of spin glasses using thermal noise: Performance of quantum annealing at finite temperatures

    NASA Astrophysics Data System (ADS)

    Nishimura, Kohji; Nishimori, Hidetoshi; Ochoa, Andrew J.; Katzgraber, Helmut G.

    2016-09-01

    We study the problem to infer the ground state of a spin-glass Hamiltonian using data from another Hamiltonian with interactions disturbed by noise from the original Hamiltonian, motivated by the ground-state inference in quantum annealing on a noisy device. It is shown that the average Hamming distance between the inferred spin configuration and the true ground state is minimized when the temperature of the noisy system is kept at a finite value, and not at zero temperature. We present a spin-glass generalization of a well-established result that the ground state of a purely ferromagnetic Hamiltonian is best inferred at a finite temperature in the sense of smallest Hamming distance when the original ferromagnetic interactions are disturbed by noise. We use the numerical transfer-matrix method to establish the existence of an optimal finite temperature in one- and two-dimensional systems. Our numerical results are supported by mean-field calculations, which give an explicit expression of the optimal temperature to infer the spin-glass ground state as a function of variances of the distributions of the original interactions and the noise. The mean-field prediction is in qualitative agreement with numerical data. Implications on postprocessing of quantum annealing on a noisy device are discussed.

  13. The fluctuations of the spin state of 3d-ions near the ``triple point''

    NASA Astrophysics Data System (ADS)

    Zhitlukhina, E. S.; Lamonova, K. V.; Orel, S. M.; Pashkevich, Yu. G.

    2012-10-01

    The spin states of 3d ions placed in an arbitrarily distorted coordination complex are investigated within the semiempirical modified crystal-field theory. A scheme for constructing spin-state diagrams is presented. Spin-state diagrams are obtained for transition metal ions with electron configurations 3d4, 3d5, and 3d6 placed in a pyramidal environment. The spin-state diagrams for all configurations studied display so-called "triple points", i.e., regions where the spin states are mixed in equal proportions. The spin-state evolution of a five-coordinated Co3+ ion in the layered rare-earth cobaltite GdBaCo2O5.5 is studied. It is found that the intermediate spin state of the Co3+ ion is stabilized by the apex oxygen displacement along the pyramidal axis.

  14. Generating spin squeezing states and Greenberger-Horne-Zeilinger entanglement using a hybrid phonon-spin ensemble in diamond

    NASA Astrophysics Data System (ADS)

    Xia, Keyu; Twamley, Jason

    2016-11-01

    Quantum squeezing and entanglement of spins can be used to improve the sensitivity in quantum metrology. Here we propose a scheme to create collective coupling of an ensemble of spins to a mechanical vibrational mode actuated by an external magnetic field. We find an evolution time where the mechanical motion decouples from the spins, and the accumulated geometric phase yields a squeezing of 5.9 dB for 20 spins. We also show the creation of a Greenberger-Horne-Zeilinger spin state for 20 spins with a fidelity of ˜0.62 at cryogenic temperature. The numerical simulations show that the geometric-phase-based scheme is mostly immune to thermal mechanical noise.

  15. Preparing arbitrary pure states of spatial qudits with a single phase-only spatial light modulator

    NASA Astrophysics Data System (ADS)

    Solís-Prosser, M. A.; Arias, A.; Varga, J. J. M.; Rebón, L.; Ledesma, S.; Iemmi, C.; Neves, L.

    2013-11-01

    Spatial qudits are D-dimensional ($D\\geq 2$) quantum systems carrying information encoded in the discretized transverse momentum and position of single photons. We present a proof-of-principle demonstration of a method for preparing arbitrary pure states of such systems by using a single phase-only spatial light modulator (SLM). The method relies on the encoding of the complex transmission function corresponding to a given spatial qudit state onto a preset diffraction order of a phase-only grating function addressed at the SLM. Fidelities of preparation above 94% were obtained with this method, which is simpler, less costly, and more efficient than those that require two SLMs for the same purpose.

  16. Preparing arbitrary pure states of spatial qudits with a single phase-only spatial light modulator.

    PubMed

    Solís-Prosser, M A; Arias, A; Varga, J J M; Rebón, L; Ledesma, S; Iemmi, C; Neves, L

    2013-11-15

    Spatial qudits are D-dimensional (D ≥ 2) quantum systems carrying information encoded in the discretized transverse momentum and position of single photons. We present a proof-of-principle demonstration of a method for preparing arbitrary pure states of such systems by using a single phase-only spatial light modulator (SLM). The method relies on the encoding of the complex transmission function corresponding to a given spatial qudit state onto a preset diffraction order of a phase-only grating function addressed at the SLM. Fidelities of preparation above 94% were obtained with this method, which is simpler, less costly, and more efficient than those that require two SLMs for the same purpose.

  17. Exploring ground states and excited states of spin-1 Bose-Einstein condensates by continuation methods

    SciTech Connect

    Chen, Jen-Hao; Chern, I-Liang; Wang Weichung

    2011-03-20

    A pseudo-arclength continuation method (PACM) is employed to compute the ground state and excited state solutions of spin-1 Bose-Einstein condensates (BEC). The BEC is governed by the time-independent coupled Gross-Pitaevskii equations (GPE) under the conservations of the mass and magnetization. The coupling constants that characterize the spin-independent and spin-exchange interactions are chosen as the continuation parameters. The continuation curve starts from a ground state or an excited state with very small coupling parameters. The proposed numerical schemes allow us to investigate the effect of the coupling constants and study the bifurcation diagrams of the time-independent coupled GPE. Numerical results on the wave functions and their corresponding energies of spin-1 BEC with repulsive/attractive and ferromagnetic/antiferromagnetic interactions are presented. Furthermore, we reveal that the component separation and population transfer between the different hyperfine states can only occur in excited states due to the spin-exchange interactions.

  18. Generation of Quality Pulses for Control of Qubit/Quantum Memory Spin States: Experimental and Simulation

    DTIC Science & Technology

    2016-09-01

    TECHNICAL REPORT 3046 September 2016 GENERATION OF QUALITY PULSES FOR CONTROL OF QUBIT/QUANTUM MEMORY SPIN STATES: EXPERIMENTAL AND SIMULATION...nuclear spin states of qubits/quantum memory applicable to semiconductor, superconductor, ionic, and superconductor-ionic hybrid technologies. As the...expected control of the spin flipping and rotation in the Bloch sphere

  19. Maximally entangled set of tripartite qutrit states and pure state separable transformations which are not possible via local operations and classical communication

    NASA Astrophysics Data System (ADS)

    Hebenstreit, M.; Spee, C.; Kraus, B.

    2016-01-01

    Entanglement is the resource to overcome the restriction of operations to local operations assisted by classical communication (LOCC). The maximally entangled set (MES) of states is the minimal set of n -partite pure states with the property that any truly n -partite entangled pure state can be obtained deterministically via LOCC from some state in this set. Hence, this set contains the most useful states for applications. In this work, we characterize the MES for generic three-qutrit states. Moreover, we analyze which generic three-qutrit states are reachable (and convertible) under LOCC transformations. To this end, we study reachability via separable operations (SEP), a class of operations that is strictly larger than LOCC. Interestingly, we identify a family of pure states that can be obtained deterministically via SEP but not via LOCC. This gives an affirmative answer to the question of whether there is a difference between SEP and LOCC for transformations among pure states.

  20. Spin-ordered ground state and thermodynamic behaviors of the spin-3/2 kagome Heisenberg antiferromagnet.

    PubMed

    Liu, Tao; Li, Wei; Su, Gang

    2016-09-01

    Three different tensor network (TN) optimization algorithms are employed to accurately determine the ground state and thermodynamic properties of the spin-3/2 kagome Heisenberg antiferromagnet. We found that the sqrt[3]×sqrt[3] state (i.e., the state with 120^{∘} spin configuration within a unit cell containing 9 sites) is the ground state of this system, and such an ordered state is melted at any finite temperature, thereby clarifying the existing experimental controversies. Three magnetization plateaus (m/m_{s}=1/3,23/27, and 25/27) were obtained, where the 1/3-magnetization plateau has been observed experimentally. The absence of a zero-magnetization plateau indicates a gapless spin excitation that is further supported by the thermodynamic asymptotic behaviors of the susceptibility and specific heat. At low temperatures, the specific heat is shown to exhibit a T^{2} behavior, and the susceptibility approaches a finite constant as T→0. Our TN results of thermodynamic properties are compared with those from high-temperature series expansion. In addition, we disclose a quantum phase transition between q=0 state (i.e., the state with 120^{∘} spin configuration within a unit cell containing three sites) and sqrt[3]×sqrt[3] state in a spin-3/2 kagome XXZ model at the critical point Δ_{c}=0.54. This study provides reliable and useful information for further explorations on high-spin kagome physics.

  1. Spin-ordered ground state and thermodynamic behaviors of the spin-3/2 kagome Heisenberg antiferromagnet

    NASA Astrophysics Data System (ADS)

    Liu, Tao; Li, Wei; Su, Gang

    2016-09-01

    Three different tensor network (TN) optimization algorithms are employed to accurately determine the ground state and thermodynamic properties of the spin-3/2 kagome Heisenberg antiferromagnet. We found that the √{3 }×√{3 } state (i.e., the state with 120° spin configuration within a unit cell containing 9 sites) is the ground state of this system, and such an ordered state is melted at any finite temperature, thereby clarifying the existing experimental controversies. Three magnetization plateaus (m /ms=1 /3 ,23 /27 , and 25/27) were obtained, where the 1/3-magnetization plateau has been observed experimentally. The absence of a zero-magnetization plateau indicates a gapless spin excitation that is further supported by the thermodynamic asymptotic behaviors of the susceptibility and specific heat. At low temperatures, the specific heat is shown to exhibit a T2 behavior, and the susceptibility approaches a finite constant as T →0 . Our TN results of thermodynamic properties are compared with those from high-temperature series expansion. In addition, we disclose a quantum phase transition between q =0 state (i.e., the state with 120° spin configuration within a unit cell containing three sites) and √{3 }×√{3 } state in a spin-3/2 kagome XXZ model at the critical point Δc=0.54 . This study provides reliable and useful information for further explorations on high-spin kagome physics.

  2. Approximating the ground state of gapped quantum spin systems

    SciTech Connect

    Michalakis, Spyridon; Hamza, Eman; Nachtergaele, Bruno; Sims, Robert

    2009-01-01

    We consider quantum spin systems defined on finite sets V equipped with a metric. In typical examples, V is a large, but finite subset of Z{sup d}. For finite range Hamiltonians with uniformly bounded interaction terms and a unique, gapped ground state, we demonstrate a locality property of the corresponding ground state projector. In such systems, this ground state projector can be approximated by the product of observables with quantifiable supports. In fact, given any subset {chi} {contained_in} V the ground state projector can be approximated by the product of two projections, one supported on {chi} and one supported on {chi}{sup c}, and a bounded observable supported on a boundary region in such a way that as the boundary region increases, the approximation becomes better. Such an approximation was useful in proving an area law in one dimension, and this result corresponds to a multi-dimensional analogue.

  3. Using corresponding state theory to obtain intermolecular potentials to calculate pure liquid shock Hugoniots

    SciTech Connect

    Hobbs, M.L.

    1997-12-01

    Determination of product species, equations-of-state (EOS) and thermochemical properties of high explosives and pyrotechnics remains a major unsolved problem. Although, empirical EOS models may be calibrated to replicate detonation conditions within experimental variability (5--10%), different states, e.g. expansion, may produce significant discrepancy with data if the basic form of the EOS model is incorrect. A more physically realistic EOS model based on intermolecular potentials, such as the Jacobs Cowperthwaite Zwisler (JCZ3) EOS, is needed to predict detonation states as well as expanded states. Predictive capability for any EOS requires a large species data base composed of a wide variety of elements. Unfortunately, only 20 species have known JCZ3 molecular force constants. Of these 20 species, only 10 have been adequately compared to experimental data such as molecular scattering or shock Hugoniot data. Since data in the strongly repulsive region of the molecular potential is limited, alternative methods must be found to deduce force constants for a larger number of species. The objective of the present study is to determine JCZ3 product species force constants by using a corresponding states theory. Intermolecular potential parameters were obtained for a variety of gas species using a simple corresponding states technique with critical volume and critical temperature. A more complex, four parameter corresponding state method with shape and polarity corrections was also used to obtain intermolecular potential parameters. Both corresponding state methods were used to predict shock Hugoniot data obtained from pure liquids. The simple corresponding state method is shown to give adequate agreement with shock Hugoniot data.

  4. Electrical control of flying spin precession in chiral 1D edge states

    SciTech Connect

    Nakajima, Takashi; Komiyama, Susumu; Lin, Kuan-Ting

    2013-12-04

    Electrical control and detection of spin precession are experimentally demonstrated by using spin-resolved edge states in the integer quantum Hall regime. Spin precession is triggered at a corner of a biased metal gate, where electron orbital motion makes a sharp turn leading to a nonadiabatic change in the effective magnetic field via spin-orbit interaction. The phase of precession is controlled by the group velocity of edge-state electrons tuned by gate bias voltage: Spin-FET-like coherent control of spin precession is thus realized by all-electrical means.

  5. Spin-polarized local density of states around vortex in helical p-wave superconductors

    NASA Astrophysics Data System (ADS)

    Tanaka, Kenta K.; Ichioka, Masanori; Onari, Seiichiro

    2017-07-01

    Based on the quasi-classical Eilenberger theory, we investigate the magnetic field dependence of order-parameters and spin-polarized local density of states (LDOS) in the vortex lattice state of helical p-wave superconductors. The spin-polarized LDOS is induced by the vorticity coupling to the chirality of up-spin pair or down-spin pair, even when Knight shift does not change. We clarify the instability of the helical p-wave state at high field, and that the spin-polarized LDOS shows the unique behaviors of the helical p-wave state.

  6. Gate-controlled switching between persistent and inverse persistent spin helix states

    SciTech Connect

    Yoshizumi, K.; Sasaki, A.; Kohda, M.; Nitta, J.

    2016-03-28

    We demonstrate gate-controlled switching between persistent spin helix (PSH) state and inverse PSH state, which are detected by quantum interference effect on magneto-conductance. These special symmetric spin states showing weak localization effect give rise to a long spin coherence when the strength of Rashba spin-orbit interaction (SOI) is close to that of Dresselhaus SOI. Furthermore, in the middle of two persistent spin helix states, where the Rashba SOI can be negligible, the bulk Dresselhaus SOI parameter in a modulation doped InGaAs/InAlAs quantum well is determined.

  7. Spin State Equilibria of Asteroids due to YORP Effects

    NASA Astrophysics Data System (ADS)

    Golubov, Oleksiy; Scheeres, Daniel J.; Lipatova, Veronika

    2016-05-01

    Spins of small asteroids are controlled by the Yarkovsky--O'Keefe--Radzievskii--Paddack (YORP) effect. The normal version of this effect has two components: the axial component alters the rotation rate, while the obliquity component alters the obliquity. Under this model the rotation state of an asteroid can be described in a phase plane with the rotation rate along the polar radius and the obliquity as the polar angle. The YORP effect induces a phase flow in this plane, which determines the distribution of asteroid rotation rates and obliquities.We study the properties of this phase flow for several typical cases. Some phase flows have stable attractors, while in others all trajectories go to very small or large rotation rates. In the simplest case of zero thermal inertia approximate analytical solutions to dynamics equations are possible. Including thermal inertia and the Tangential YORP effect makes the possible evolutionary scenarios much more diverse. We study possible evolution paths and classify the most general trends. Also we discuss possible implications for the distribution of asteroid rotation rates and obliquities.A special emphasis is put on asteroid (25143) Itokawa, whose shape model is well determined, but who's measured YORP acceleration does not agree with the predictions of normal YORP. We show that Itokawa's rotational state can be explained by the presence of tangential YORP and that it may be in or close to a stable spin state equilibrium. The implications of such states will be discussed.

  8. Svetlichny's inequality and genuine tripartite nonlocality in three-qubit pure states

    SciTech Connect

    Ajoy, Ashok; Rungta, Pranaw

    2010-05-15

    The violation of the Svetlichny's inequality (SI) [Phys. Rev. D 35, 3066 (1987)] is sufficient but not necessary for genuine tripartite nonlocal correlations. Here we quantify the relationship between tripartite entanglement and the maximum expectation value of the Svetlichny operator (which is bounded from above by the inequality) for the two inequivalent subclasses of pure three-qubit states: the Greenberger-Horne-Zeilinger (GHZ) class and the W class. We show that the maximum for the GHZ-class states reduces to Mermin's inequality [Phys. Rev. Lett. 65, 1838 (1990)] modulo a constant factor, and although it is a function of the three tangle and the residual concurrence, large numbers of states do not violate the inequality. We further show that by design SI is more suitable as a measure of genuine tripartite nonlocality between the three qubits in the W-class states, and the maximum is a certain function of the bipartite entanglement (the concurrence) of the three reduced states, and only when their sum attains a certain threshold value do they violate the inequality.

  9. Magnetic transitions and Fe(II) spin state in mackinawite

    NASA Astrophysics Data System (ADS)

    Schroeder, C.; Wan, M.; Peiffer, S.

    2012-12-01

    (S=1) state, but not high spin (S=2). Paramagnetic substances which become magnetically ordered below a certain temperature must have unpaired electrons (S≠0). Fe(II) in mackinawite is tetrahedrally coordinated to S, and frontier molecular orbital theory modeling suggests Fe to be either in intermediate spin (S=1) or high spin (S=2) state [7]. Combined with Mössbauer isomer shifts, Fe(II) in mackinawite must therefore be in the intermediate spin (S=1) state. The absence of magnetic ordering in the freshly precipitated and filtered mackinawite sample can be explained by either extremely small particle size resulting in superparamagnetic behavior, or Fe(II) is in a low spin (S=0) state and therefore diamagnetic. In the latter case this phase cannot be mackinawite but may be cubic FeSc, the Fe equivalent of sphalerite (cubic ZnS). References: [1] Wan et al., Mineral. Mag. 75(3) (2011) 2112. [2] Wan et al., Geophysical Research Abstracts 14, EGU2012-4724-3. [3] Hellige et al., Geochim. Cosmochim. Ac. 81 (2012) 69-81. [4] Morice et al., J. inorg. nucl. Chem. 31 (1969) 3797-3802. [5] Vaughan and Ridout, J. inorg. nucl. Chem. 33 (1971) 741-746. [6] Mullet et al., Geochim. Cosmochim. Ac. 66 (2002) 829-836. [7] Luther III, personal communication.

  10. Cortical activation in response to pure taste stimuli during the physiological states of hunger and satiety.

    PubMed

    Haase, Lori; Cerf-Ducastel, Barbara; Murphy, Claire

    2009-02-01

    This event-related functional magnetic resonance imaging (er-fMRI) study investigated BOLD signal change in response to a series of pure gustatory stimuli that varied in stimulus quality when subjects were hungry and sated with a nutritional pre-load. Group analyses showed significant differences in activation in the hunger minus satiety condition in response to sucrose, caffeine, saccharin, and citric acid within the thalamus, hippocampus, and parahippocampus. When examining the hunger and satiety conditions, activation varied as a function of stimulus, with the majority of the stimuli exhibiting significantly greater activation in the hunger state within the insula, thalamus, and substantia nigra, in contrast to decreased activation in the satiated state within the parahippocampus, hippocampus, amygdala, and anterior cingulate. Region of interest (ROI) analysis revealed two significant interactions, ROI by physiology and ROI by physiology by stimulus. In the satiety condition, the primary (inferior and superior insulae) and secondary (OFC 11 and OFC 47) taste regions exhibited significantly greater brain activation in response to all stimuli than regions involved in processing eating behavior (hypothalamus), affect (amygdala), and memory (hippocampus, parahippocampus and entorhinal cortex). These same regions demonstrated significantly greater activation within the hunger condition than the satiety condition, with the exception of the superior insula. Furthermore, the patterns of activation differed as a function taste stimulus, with greater activation in response to sucrose than to the other stimuli. These differential patterns of activation suggest that the physiological states of hunger and satiety produce divergent activation in multiple brain areas in response to different pure gustatory stimuli.

  11. Collectivity of high spin states in {sup 84}Zr

    SciTech Connect

    Lister, C.J.; Blumenthal, D.; Crowell, B.

    1995-08-01

    {sup 84}Zr is one of the most extensively studied of the A {approximately} 80 rotors, both from theoretical and experimental approaches. It was predicted to be a good candidate to support superdeformation, and to show interesting spectroscopic properties including saturation of its shell-model space at lower spin. We performed an experiment using Gammasphere in its early implementation phase. The reaction of {sup 29}Si on {sup 58}Ni was used to strongly populate {sup 84}Zr at high spin. Thin and thick targets were used to allow the extraction of transitional matrix elements at very high spin, and to allow a sensitive search for superdeformed states. Data analysis is in progress. The large data set allowed us to extend the previously known bands considerably. Candidates for a staggered M1-band, found previously {sup 86}Zr, were located. To date, no evidence for superdeformed bands was found. Analysis was slowed by the relocation of all the participants in this experiment, but we hope to complete the lifetime analysis this year. This analysis has become especially topical, due to reported measurements of superdeformation in this region.

  12. Ground states, magnetization plateaus and bipartite entanglement of frustrated spin-1/2 Ising-Heisenberg and Heisenberg triangular tubes

    NASA Astrophysics Data System (ADS)

    Alécio, Raphael C.; Lyra, Marcelo L.; Strečka, Jozef

    2016-11-01

    The ground-state phase diagram, magnetization process and bipartite entanglement of the frustrated spin-1/2 Ising-Heisenberg and Heisenberg triangular tube (three-leg ladder) are investigated in a non-zero external magnetic field. The exact ground-state phase diagram of the spin-1/2 Ising-Heisenberg tube with Heisenberg intra-rung and Ising inter-rung couplings consists of six distinct gapped phases, which manifest themselves in a magnetization curve as intermediate plateaus at zero, one-third and two-thirds of the saturation magnetization. Four out of six available ground states exhibit quantum entanglement between two spins from the same triangular unit evidenced by a non-zero concurrence. Density-matrix renormalization group calculations are used in order to construct the ground-state phase diagram of the analogous but purely quantum spin-1/2 Heisenberg tube with Heisenberg intra- and inter-rung couplings, which consists of four gapped and three gapless phases. The Heisenberg tube shows a continuous change of the magnetization instead of a plateau at zero magnetization, while the intermediate one-third and two-thirds plateaus may be present or not in the zero-temperature magnetization curve.

  13. Measurements of Mercury's spin state and inferences about its interior

    NASA Astrophysics Data System (ADS)

    Margot, J.; Padovan, S.; Peale, S. J.; Solomon, S. C.

    2011-12-01

    Over the past nine years we have used the Green Bank Telescope (GBT) in conjunction with the Goldstone Solar System Radar (GSSR) to characterize the spin state and interior of Mercury. We implemented a technique [1,2] that provides instantaneous spin rate measurements with 10-5 fractional precision and spin orientation measurements at the arcsecond level. On the basis of measurements at 21 distinct epochs between 2002 and 2006, we found observational evidence that Mercury closely follows a Cassini state and that it exhibits forced librations in longitude [3], as predicted by theory [4,5]. A long-period (˜12 year) libration signature may be present in the data. Since 2006 we have secured measurements at 11 additional epochs (out of 23 attempts). We are in the process of re-analyzing the entire set of observations with the goals of (1) refining the determination of the obliquity and of the libration amplitude, two parameters that are critical in the determination of the core size; (2) confirming the presence or absence of a long-period libration component, with the prospect of elucidating the excitation mechanism; (3) quantifying deviations of the pole from the strict Cassini state, which could inform us about dissipation due to solid-body tides and core-mantle interactions. Our first goal is particularly important now that MESSENGER is securing measurements of the low-degree gravitational harmonics with an expected precision of better than 1%. The core-size error budget indicates that the precision of the ground-based estimates of obliquity and librations will ultimately dictate the quality of the core size determination, as well as the attendant inferences regarding the interior structure, thermal evolution, and magnetic field generation of the planet. [1] Green, in Radar Astronomy, McGraw-Hill, 1968. [2] Holin, Radiophys. Quant. Elec. 31, 1988. [3] Margot et al, Science 316, 2007. [4] Peale, Nature 262, 1976. [5] Peale, in Mercury, U. of Arizona Press, 1988.

  14. A quantum phase switch between a single solid-state spin and a photon.

    PubMed

    Sun, Shuo; Kim, Hyochul; Solomon, Glenn S; Waks, Edo

    2016-06-01

    Interactions between single spins and photons are essential for quantum networks and distributed quantum computation. Achieving spin-photon interactions in a solid-state device could enable compact chip-integrated quantum circuits operating at gigahertz bandwidths. Many theoretical works have suggested using spins embedded in nanophotonic structures to attain this high-speed interface. These proposals implement a quantum switch where the spin flips the state of the photon and a photon flips the spin state. However, such a switch has not yet been realized using a solid-state spin system. Here, we report an experimental realization of a spin-photon quantum switch using a single solid-state spin embedded in a nanophotonic cavity. We show that the spin state strongly modulates the polarization of a reflected photon, and a single reflected photon coherently rotates the spin state. These strong spin-photon interactions open up a promising direction for solid-state implementations of high-speed quantum networks and on-chip quantum information processors using nanophotonic devices.

  15. Preparation and coherent manipulation of pure quantum states of a single molecular ion

    NASA Astrophysics Data System (ADS)

    Chou, Chin-Wen; Kurz, Christoph; Hume, David B.; Plessow, Philipp N.; Leibrandt, David R.; Leibfried, Dietrich

    2017-05-01

    Laser cooling and trapping of atoms and atomic ions has led to advances including the observation of exotic phases of matter, the development of precision sensors and state-of-the-art atomic clocks. The same level of control in molecules could also lead to important developments such as controlled chemical reactions and sensitive probes of fundamental theories, but the vibrational and rotational degrees of freedom in molecules pose a challenge for controlling their quantum mechanical states. Here we use quantum-logic spectroscopy, which maps quantum information between two ion species, to prepare and non-destructively detect quantum mechanical states in molecular ions. We develop a general technique for optical pumping and preparation of the molecule into a pure initial state. This enables us to observe high-resolution spectra in a single ion (CaH+) and coherent phenomena such as Rabi flopping and Ramsey fringes. The protocol requires a single, far-off-resonant laser that is not specific to the molecule, so many other molecular ions, including polyatomic species, could be treated using the same methods in the same apparatus by changing the molecular source. Combined with the long interrogation times afforded by ion traps, a broad range of molecular ions could be studied with unprecedented control and precision. Our technique thus represents a critical step towards applications such as precision molecular spectroscopy, stringent tests of fundamental physics, quantum computing and precision control of molecular dynamics.

  16. The excited spin state of Comet 2P/Encke

    NASA Astrophysics Data System (ADS)

    Belton, Michael J. S.; Samarasinha, Nalin H.; Fernández, Yan R.; Meech, Karen J.

    2005-05-01

    Ways to rationalize the different periods (e.g., 15.08 h, Luu and Jewitt, 1990, Icarus 86, 69-81; 11.01 h, Fernández et al., 2004, Icarus, in this issue; Lowry et al., 2003, Lunar Planet. Sci. XXXIV, Abstract 2056) seen in near aphelion R-band light curves of Comet 2P/Encke are explored. We show that the comet is usually active at aphelion and it's observed light curves contain signal from both the nucleus and an unresolved coma. The coma contribution to the observed brightness is generally found to dominate with the nucleus providing from 28 to 87% of the total brightness. The amplitude of the observed variations cannot be explained by the nucleus alone and are due to coma activity. We show that some seven periodicities exist in the observed light curves at various times and that this is likely the result of an active nucleus spinning in an excited spin state. The changing periodicities are probably due to changes in the relative strengths of the active areas. We work out possible excited states based on experience with model light curves and by using an analogy to light curve observations of Comet 1P/Halley for which the spin state has been separately determined from spacecraft observations. There is a possibility of a fully relaxed principal axis spin state (0.538 d -1; P=44.6 h) but, because it provides a poorer fit to the observed periodicities than the best fit excited state together with the absence of a peak near 1.08 d -1 ( 2f) in the frequency spectrum of the Fernández et al. (2000, Icarus 147, 145-160) thermal IR lightcurve, we consider it unlikely. Both SAM and LAM excited states are allowed by the underlying periodicities and additional information is needed to choose between these. Our choice of a low excitation SAM state, i.e., one in which the instantaneous spin axis nutates around the total angular momentum vector in a motion that is characterized by limited angular oscillations around the long axis, is based on Sekanina's (1988, Astron J. 95

  17. Spin polarized photoemission studies of magnetic quantum well states

    SciTech Connect

    Johnson, P.D.

    1994-12-01

    There is currently considerable technological interest in the properties of transition metal multilayers. In these multilayers, which include Fe/Cr(001) and Cu/Co(001), it is possible to achieve either ferromagnetic or antiferromagnetic coupling of the adjacent ferromagnetic layers depending on the thickness of the intervening layer. The related giant magnetoresistance properties and the large enhancement of the Kerr rotation in these systems make them particularly interesting. In this paper, quantum well states with discrete binding energies dependent on the thickness of the film are observed in copper films deposited on a Co(001) substrate. They are found to be spin polarized, preferentially with minority spin. These states pass up to and through the Fermi level with a frequency identical to the long period of oscillation in the associated magnetic multilayers. In the pre-asymptotic limit the dispersion of these states away from the center of the zone is described by enhanced effective masses. This has implications for theories of the oscillatory exchange coupling that invoke the bulk Fermi surface.

  18. Spin-state-correlated optical properties of copper(ii)-nitroxide based molecular magnets.

    PubMed

    Barskaya, Irina Yu; Veber, Sergey L; Suturina, Elizaveta A; Sherin, Peter S; Maryunina, Kseniya Yu; Artiukhova, Natalia A; Tretyakov, Evgeny V; Sagdeev, Renad Z; Ovcharenko, Victor I; Gritsan, Nina P; Fedin, Matvey V

    2017-10-03

    Molecular magnets based on copper(ii) ions and stable nitroxide radicals exhibit promising switchable behavior triggered by a number of external stimuli; however, their spin-state-correlated optical properties vital for photoinduced switching have not been profoundly investigated to date. Herein, the electronic absorption spectra of single crystals of three representatives of this unique family are studied experimentally and theoretically in the visible and near-IR regions. We established that the color of the complexes is mainly determined by optical properties of the nitroxide radicals, whereas the Cu(hfac)2 fragment contributes to the near-IR range with the intensity smaller by an order of magnitude. The thermochromism of these complexes evident upon thermal spin state switching is mainly caused by a spectral shift of the absorption bands of the nitroxides. The vibrational progression observed in the visible range for single crystals as well as for solutions of pure nitroxides is well reproduced by DFT calculations, where the C-C stretching mode governs the observed progression. The analysis of the spectra of single crystals in the near-IR region reveals changes in the energy and in the intensity of the copper(ii) d-d transitions, which are well reproduced by SOC-NEVPT2 calculations and owe to the flip of the Jahn-Teller axis in the coordination environment of copper. Further strategies for designing bidirectional magnetic photoswitches using these appealing compounds are discussed.

  19. Coherent manipulation, measurement and entanglement of individual solid-state spins using optical fields

    NASA Astrophysics Data System (ADS)

    Gao, W. B.; Imamoglu, A.; Bernien, H.; Hanson, R.

    2015-06-01

    Realization of a quantum interface between stationary and flying qubits is a requirement for long-distance quantum communication and distributed quantum computation. The prospects for integrating many qubits on a single chip render solid-state spins promising candidates for stationary qubits. Certain solid-state systems, including quantum dots and nitrogen-vacancy centres in diamond, exhibit spin-state-dependent optical transitions, allowing for fast initialization, manipulation and measurement of the spins using laser excitation. Recent progress has brought spin photonics research in these materials into the quantum realm, allowing the demonstration of spin-photon entanglement, which in turn has enabled distant spin entanglement as well as quantum teleportation. Advances in the fabrication of photonic nanostructures hosting spin qubits suggest that chips incorporating a high-efficiency spin-photon interface in a quantum photonic network are within reach.

  20. Theoretical Study of Renewable Ionic Liquids in the Pure State and with Graphene and Carbon Nanotubes.

    PubMed

    García, Gregorio; Atilhan, Mert; Aparicio, Santiago

    2015-09-17

    The N-ethyl-N-(furan-2-ylmethyl)ethanaminium dihydrogen phosphate ionic liquid was studied as a model of ionic liquids which can be produced from totally renewable sources. A computational study using both molecular dynamics and density functional theory methods was carried out. The properties, structuring, and intermolecular interactions (hydrogen bonding) of this fluid in the pure state were studied as a function of pressure and temperature. Likewise, the adsorption on graphene and the confinement between graphene sheets was also studied. The solvation of single walled carbon nanotubes in the selected ionic liquid was analyzed together with the behavior of ions confined inside these nanotubes. The reported results show remarkable properties for this fluid, which show that many of the most relevant properties of ionic liquids and their ability to interact with carbon nanosystems may be maintained and even improved using new families of renewable compounds instead of classic types of ionic liquids with worse environmental, toxicological, and economical profiles.

  1. Charge transfer states appear in the π-conjugated pure hydrocarbon molecule on Cu(111)

    NASA Astrophysics Data System (ADS)

    Yonezawa, Keiichirou; Suda, Yosuke; Yanagisawa, Susumu; Hosokai, Takuya; Kato, Kengo; Yamaguchi, Takuma; Yoshida, Hiroyuki; Ueno, Nobuo; Kera, Satoshi

    2016-04-01

    We report on the results of experimental and theoretical studies on the electronic structure of gas-phase diindenoperylene (DIP) and DIP-monolayer (ML) on Cu(111). Vapor-phase ultraviolet photoelectron spectroscopy (UPS) was realized for 11.3 mg of DIP, giving reference orbital energies of isolated DIP, and UPS and inverse photoemission spectroscopy of DIP-ML/graphite were performed to obtain DIP-ML electronic states at a weak interfacial interaction. Furthermore, first-principles calculation clearly demonstrates the interfacial rearrangement. These results provide evidence that the rearrangement of orbital energies, which is realized in HOMO-LUMO and HOMO-HOMO-1 gaps, brings partially occupied LUMO through the surface-induced aromatic stabilization of DIP, a pure hydrocarbon molecule, on Cu(111).

  2. Entropy-power uncertainty relations: towards a tight inequality for all Gaussian pure states

    NASA Astrophysics Data System (ADS)

    Hertz, Anaelle; Jabbour, Michael G.; Cerf, Nicolas J.

    2017-09-01

    We show that a proper expression of the uncertainty relation for a pair of canonically-conjugate continuous variables relies on entropy power, a standard notion in Shannon information theory for real-valued signals. The resulting entropy-power uncertainty relation is equivalent to the entropic formulation of the uncertainty relation due to Bialynicki-Birula and Mycielski, but can be further extended to rotated variables. Hence, based on a reasonable assumption, we give a partial proof of a tighter form of the entropy-power uncertainty relation taking correlations into account and provide extensive numerical evidence of its validity. Interestingly, it implies the generalized (rotation-invariant) Schrödinger-Robertson uncertainty relation exactly as the original entropy-power uncertainty relation implies Heisenberg relation. It is saturated for all Gaussian pure states, in contrast with hitherto known entropic formulations of the uncertainty principle.

  3. Spin-Resolved Photoemission of Surface States of W(110)-(1×1)H

    NASA Astrophysics Data System (ADS)

    Hochstrasser, M.; Tobin, J. G.; Rotenberg, Eli; Kevan, S. D.

    2002-11-01

    The surface electronic states of W(110)-(1×1)H have been measured using spin- and angle-resolved photoemission. We directly demonstrate that the surface bands are both split and spin-polarized by the spin-orbit interaction in association with the loss of inversion symmetry near a surface. We observe 100% spin polarization of the surface states, with the spins aligned in the plane of the surface and oriented in a circular fashion relative to the S¯ symmetry point. In contrast, no measurable polarization of nearby bulk states is observed.

  4. Numerical Modeling of the Central Spin Problem Using the Spin-Coherent-State P Representation

    SciTech Connect

    Al Hassanieh, Khaled A; Dobrovitski, V. V.; Dagotto, Elbio R; Harmon, B. N.

    2006-01-01

    In this work, we consider decoherence of a central spin by a spin bath. In order to study the nonperturbative decoherence regimes, we develop an efficient mean-field-based method for modeling the spin-bath decoherence, based on the P representation of the central spin density matrix. The method can be applied to longitudinal and transverse relaxation at different external fields. In particular, by modeling large-size quantum systems (up to 16 000 bath spins), we make controlled predictions for the slow long-time decoherence of the central spin.

  5. Spin-pseudospin intertwined excitation at the ν = 1 bilayer quantum Hall state investigated by nuclear-spin relaxation

    SciTech Connect

    Tsuda, S.; Nguyen, M. H.; Terasawa, D.; Fukuda, A.; Zheng, Y. D.; Arai, T.; Sawada, A.; Ezawa, Z. F.

    2013-12-04

    We investigate the electron spin degree of freedom at the imbalanced density bilayer ν = 1 quantum Hall states using the resistively detected nuclear-spin-lattice relaxation rate 1/T{sub 1}. Our measurements reveal a continuous change in 1/T{sub 1} for σ = 1 to 0, suggesting that the balanced density ν = 1 state also exhibits electron-spin fluctuations. Moreover, the value of 1/T{sub 1} in the back layer (the layer from which electrons are transferred to the front layer) increases at intermediate density imbalance states. This indicates that the low-energy electron-spin mode, similar to a mode observed in Skyrmion crystals, might extend across the two layers.

  6. π-electron S = ½ quantum spin-liquid state in an ionic polyaromatic hydrocarbon

    NASA Astrophysics Data System (ADS)

    Takabayashi, Yasuhiro; Menelaou, Melita; Tamura, Hiroyuki; Takemori, Nayuta; Koretsune, Takashi; Štefančič, Aleš; Klupp, Gyöngyi; Buurma, A. Johan C.; Nomura, Yusuke; Arita, Ryotaro; Arčon, Denis; Rosseinsky, Matthew J.; Prassides, Kosmas

    2017-07-01

    Molecular solids with cooperative electronic properties based purely on π electrons from carbon atoms offer a fertile ground in the search for exotic states of matter, including unconventional superconductivity and quantum magnetism. The field was ignited by reports of high-temperature superconductivity in materials obtained by the reaction of alkali metals with polyaromatic hydrocarbons, such as phenanthrene and picene, but the composition and structure of any compound in this family remained unknown. Here we isolate the binary caesium salts of phenanthrene, Cs(C14H10) and Cs2(C14H10), to show that they are multiorbital strongly correlated Mott insulators. Whereas Cs2(C14H10) is diamagnetic because of orbital polarization, Cs(C14H10) is a Heisenberg antiferromagnet with a gapped spin-liquid state that emerges from the coupled highly frustrated Δ-chain magnetic topology of the alternating-exchange spiral tubes of S = ½ (C14H10)•- radical anions. The absence of long-range magnetic order down to 1.8 K (T/J ≈ 0.02 J is the dominant exchange constant) renders the compound an excellent candidate for a spin-½ quantum-spin liquid (QSL) that arises purely from carbon π electrons.

  7. Observation of spin-charge separation and boundary bound states via the local density of states

    NASA Astrophysics Data System (ADS)

    Schoenauer, Benedikt; Schmitteckert, Peter; Schuricht, Dirk

    2017-05-01

    We numerically calculate the local density of states (LDOS) of a one-dimensional Mott insulator with open boundaries, which is modelled microscopically by a (extended) Hubbard chain at half filling. In the Fourier transform of the LDOS we identify several dispersing features corresponding to propagating charge and spin degrees of freedom, thus providing a visualization of the spin-charge separation in the system. We also consider the effect of an additional boundary potential, which, if sufficiently strong, leads to the formation of a boundary bound state which is clearly visible in the LDOS as a nondispersing feature inside the Mott gap.

  8. High-spin states in 29Al and 27Mg

    NASA Astrophysics Data System (ADS)

    Dungan, R.; Tabor, S. L.; Lubna, R. S.; Volya, A.; Tripathi, Vandana; Abromeit, B.; Caussyn, D. D.; Kravvaris, K.; Tai, P.-L.

    2016-12-01

    The structure of 29Al and 27Mg was investigated using the reactions 18O(14C,p 2 n ) and 18O(14C,α n ) at 40 MeV. The charged particles were detected and identified with a Δ E -E telescope in coincidence with γ radiation detected in the Florida State University Compton suppressed γ detector array. The level and decay schemes of both nuclei have been expanded at higher spins and excitation energies. The positive-parity states up to 3.5-4.5 MeV agree well with shell model calculations using the USDA interaction. The negative-parity states in 27Mg are reproduced relatively well by one-particle-one-hole calculations with the WBP-a interaction. Three 27Mg states unbound by 0.4-1.4 MeV to neutron decay were observed to decay radiatively. One of these states had been previously observed to γ decay in a (d ,p γ ) experiment along with a surprising 16 other neutron unbound states. The competition between neutron and γ decay in these states is discussed in terms of angular momentum barriers and spectroscopic factors.

  9. Characterizing Resting-State Brain Function Using Arterial Spin Labeling

    PubMed Central

    Jann, Kay; Wang, Danny J.J.

    2015-01-01

    Abstract Arterial spin labeling (ASL) is an increasingly established magnetic resonance imaging (MRI) technique that is finding broader applications in studying the healthy and diseased brain. This review addresses the use of ASL to assess brain function in the resting state. Following a brief technical description, we discuss the use of ASL in the following main categories: (1) resting-state functional connectivity (FC) measurement: the use of ASL-based cerebral blood flow (CBF) measurements as an alternative to the blood oxygen level-dependent (BOLD) technique to assess resting-state FC; (2) the link between network CBF and FC measurements: the use of network CBF as a surrogate of the metabolic activity within corresponding networks; and (3) the study of resting-state dynamic CBF-BOLD coupling and cerebral metabolism: the use of dynamic CBF information obtained using ASL to assess dynamic CBF-BOLD coupling and oxidative metabolism in the resting state. In addition, we summarize some future challenges and interesting research directions for ASL, including slice-accelerated (multiband) imaging as well as the effects of motion and other physiological confounds on perfusion-based FC measurement. In summary, this work reviews the state-of-the-art of ASL and establishes it as an increasingly viable MRI technique with high translational value in studying resting-state brain function. PMID:26106930

  10. Characterizing Resting-State Brain Function Using Arterial Spin Labeling.

    PubMed

    Chen, J Jean; Jann, Kay; Wang, Danny J J

    2015-11-01

    Arterial spin labeling (ASL) is an increasingly established magnetic resonance imaging (MRI) technique that is finding broader applications in studying the healthy and diseased brain. This review addresses the use of ASL to assess brain function in the resting state. Following a brief technical description, we discuss the use of ASL in the following main categories: (1) resting-state functional connectivity (FC) measurement: the use of ASL-based cerebral blood flow (CBF) measurements as an alternative to the blood oxygen level-dependent (BOLD) technique to assess resting-state FC; (2) the link between network CBF and FC measurements: the use of network CBF as a surrogate of the metabolic activity within corresponding networks; and (3) the study of resting-state dynamic CBF-BOLD coupling and cerebral metabolism: the use of dynamic CBF information obtained using ASL to assess dynamic CBF-BOLD coupling and oxidative metabolism in the resting state. In addition, we summarize some future challenges and interesting research directions for ASL, including slice-accelerated (multiband) imaging as well as the effects of motion and other physiological confounds on perfusion-based FC measurement. In summary, this work reviews the state-of-the-art of ASL and establishes it as an increasingly viable MRI technique with high translational value in studying resting-state brain function.

  11. Attainability of the quantum information bound in pure-state models

    NASA Astrophysics Data System (ADS)

    Toscano, Fabricio; Bastos, Wellison P.; de Matos Filho, Ruynet L.

    2017-04-01

    The attainability of the quantum Cramér-Rao bound (QCR), the ultimate limit in the precision of the estimation of a physical parameter, requires the saturation of the quantum information bound (QIB). This occurs when the Fisher information associated to a given measurement on the quantum state of a system which encodes the information about the parameter coincides with the quantum Fisher information associated to that quantum state. Braunstein and Caves [Phys. Rev. Lett. 72, 3439 (1994), 10.1103/PhysRevLett.72.3439] have shown that the QIB can always be achieved via a projective measurement in the eigenvectors basis of an observable called the symmetric logarithmic derivative. However, such projective measurement depends, in general, on the value of the parameter to be estimated, therefore requiring previous knowledge of the quantity one is trying to estimate. For this reason, it is important to investigate under which situation it is possible to saturate the QCR without previous information about the parameter to be estimated. Here, we show the complete solution to the problem of which are the initial pure states and which projective measurements allow the global saturation of the QIB, without the knowledge of the true value of the parameter, when the information about the parameter is encoded in the system by a unitary process.

  12. Association equation of state (AEOS) based on aggregate formation for pure substance

    NASA Astrophysics Data System (ADS)

    Mohsen-Nia, M.; Modarress, H.

    2007-07-01

    Based on the statistical mechanical theories and by using the concept of grand canonical ensemble a new equation of state for aggregate formations in the association fluids has been proposed. The compressibility factor for aggregate formation in an association fluid is represented by the following equation: Z=Z+Z-1 where Zagg is the aggregate compressibility factor due to aggregate formation by hydrogen bonding of molecules and Zdis is the dispersed compressibility factor due to dispersion interactions. Each aggregate is considered as an open system in the grand canonical ensemble in which a molecule can enter to form a larger aggregate or leave to form a smaller aggregate. The average number of molecules in an aggregate is used to obtain the compressibility factor Zagg and M4 equation of state previously proposed by Mohsen-Nia et al. [M. Mohsen-Nia, H. Modarress, G.A. Mansoori, Fluid Phase Equilibr. 206 (2003) 27.] for non-association compounds is used to obtain Zdis. The obtained new association equation of state (AEOS) based on the proposed compressibility factor is used for saturated properties calculations of pure well-known association fluids: water, ammonia and methanol. The results indicate that the saturated properties are well correlated by the new AEOS with a reasonable average number of molecules in each aggregate which is in agreement with spectroscopic experimental data and ab initio calculations.

  13. Bending strain engineering in quantum spin hall system for controlling spin currents

    NASA Astrophysics Data System (ADS)

    Huang, Bing; Jin, Kyung-Hwan; Cui, Bin; Zhai, Feng; Mei, Jiawei; Liu, Feng

    2017-06-01

    Quantum spin Hall system can exhibit exotic spin transport phenomena, mediated by its topological edge states. Here the concept of bending strain engineering to tune the spin transport properties of a quantum spin Hall system is demonstrated. We show that bending strain can be used to control the spin orientation of counter-propagating edge states of a quantum spin system to generate a non-zero spin current. This physics mechanism can be applied to effectively tune the spin current and pure spin current decoupled from charge current in a quantum spin Hall system by control of its bending curvature. Furthermore, the curved quantum spin Hall system can be achieved by the concept of topological nanomechanical architecture in a controllable way, as demonstrated by the material example of Bi/Cl/Si(111) nanofilm. This concept of bending strain engineering of spins via topological nanomechanical architecture affords a promising route towards the realization of topological nano-mechanospintronics.

  14. Bending strain engineering in quantum spin hall system for controlling spin currents.

    PubMed

    Huang, Bing; Jin, Kyung-Hwan; Cui, Bin; Zhai, Feng; Mei, Jiawei; Liu, Feng

    2017-06-16

    Quantum spin Hall system can exhibit exotic spin transport phenomena, mediated by its topological edge states. Here the concept of bending strain engineering to tune the spin transport properties of a quantum spin Hall system is demonstrated. We show that bending strain can be used to control the spin orientation of counter-propagating edge states of a quantum spin system to generate a non-zero spin current. This physics mechanism can be applied to effectively tune the spin current and pure spin current decoupled from charge current in a quantum spin Hall system by control of its bending curvature. Furthermore, the curved quantum spin Hall system can be achieved by the concept of topological nanomechanical architecture in a controllable way, as demonstrated by the material example of Bi/Cl/Si(111) nanofilm. This concept of bending strain engineering of spins via topological nanomechanical architecture affords a promising route towards the realization of topological nano-mechanospintronics.

  15. Ferromagnetism in the Hubbard model: Spin waves and instability of the Nagaoka state

    NASA Astrophysics Data System (ADS)

    Wurth, P.; Müller-Hartmann, E.

    We discuss two single spin flip variational wave functions describing spin wave excitations which were proposed earlier by Shastry, Krishnamurthy and Anderson (SKA) and by Basile and Elser (BE), respectively, in order to investigate the instability of the fully polarized ferromagnetic state (Nagaoka state) in the infinite U Hubbard model. We calculate the energy of these variational states for the square lattice and for multiple chains. At the zone boundary in the vicinity of the point (0, ) the spin wave energy is reduced substantially by the binding of the spin up hole to the flipped down spin. For the square lattice this leads to a critical hole density of cr = 0.407 for the SKA spin wave and of cr = 0.322 for the BE spin wave which implies remarkable improvements in comparison to the corresponding scattering states investigated previously.

  16. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    DOE PAGES

    Jiang, Zilong; Chang, Cui -Zu; Masir, Massoud Ramezani; ...

    2016-05-04

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1–x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1–x)2Te3 into a bulk insulator, amore » large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. Lastly, the enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.« less

  17. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    NASA Astrophysics Data System (ADS)

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-05-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1-x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.

  18. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    PubMed Central

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-01-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1−x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1−x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics. PMID:27142594

  19. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states.

    PubMed

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S; MacDonald, Allan H; Shi, Jing

    2016-05-04

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1-x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.

  20. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    SciTech Connect

    Jiang, Zilong; Chang, Cui -Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-05-04

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1–x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1–x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. Lastly, the enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.

  1. Evidence of unusual spin polarization of the surface states of W(110) surface

    NASA Astrophysics Data System (ADS)

    Biswas, Deep Narayan; Mandal, Partha Sarathi; Varier, Shyama R.; Sahadev, Nishaina; Maiti, Kalobaran

    2013-02-01

    We studied the surface electronic structure of W(110) surface employing spin and angle resolved photoemission spectroscopy. Experimental results exhibit highly dispersive linear bands corresponding to the surface states and signature of Dirac cones. Spin resolved spectra exhibit unusual spin character of the energy bands and signature of time reversal symmetry breaking in some cases.

  2. Nuclear structure and high-spin states of 137Pr

    NASA Astrophysics Data System (ADS)

    Dragulescu, E.; Ivascu, M.; Petrache, C.; Popescu, D.; Semenescu, G.; Gurgu, I.; Ionescu-Bujor, M.; Iordachescu, A.; Pascovici, G.; Meyer, R. A.; Lopac, V.; Brant, S.; Paar, V.; Vorkapić, D.; Vretenar, D.

    1992-10-01

    Levels in 137Pr were populated in the 126Te( 14N, 3n) and 122Sn( 19F, 4n) reactions and the subsequent radiation was studied using in-beam γ-ray spectroscopy methods including γ-ray excitation-function, angular-distribution, γγ( t) coincidence and γ( t) measurements. A level scheme with new states up to spin {35}/{2} belonging to 137Pr is given. The lifetime of the {11}/{21} state at 563.4 keV has been determined as T {1}/{2} = 2.66±0.07 μ s. The calculation of low-lying levels in 137Pr performed in IBFM has been compared to experimental data.

  3. Natural reference for nuclear high-spin states

    SciTech Connect

    Rowley, Neil; Ollier, James; Simpson, John

    2009-08-15

    We suggest two new representations of the data on rotational nuclei. The first is reference-free and the second arises from a natural reference related to the variable moment of inertia model parameters of the ground-state band of the system. As such, neither representation contains any free parameters. By defining a 'configuration spin' we show how a new ground-state band reference can be applied. Its use allows a complete description of the changes associated with the first, and higher, band crossings. We apply these new representations to discuss the nature of the first band crossing along even-even isotopic chains in the erbium and osmium isotopes and to odd-even nuclei in the vicinity of {sup 158}Er.

  4. Spin mapping of surface and bulk Rashba states in ferroelectric α -GeTe(111) films

    NASA Astrophysics Data System (ADS)

    Elmers, H. J.; Wallauer, R.; Liebmann, M.; Kellner, J.; Morgenstern, M.; Wang, R. N.; Boschker, J. E.; Calarco, R.; Sánchez-Barriga, J.; Rader, O.; Kutnyakhov, D.; Chernov, S. V.; Medjanik, K.; Tusche, C.; Ellguth, M.; Volfova, H.; Borek, St.; Braun, J.; Minár, J.; Ebert, H.; Schönhense, G.

    2016-11-01

    The breaking of bulk inversion symmetry in ferroelectric semiconductors causes a Rashba-type spin splitting of electronic bulk bands. This is shown by a comprehensive mapping of the spin polarization of the electronic bands in ferroelectric α -GeTe(111) films using a time-of-flight momentum microscope equipped with an imaging spin filter that enables a simultaneous measurement of more than 10 000 data points. The experiment reveals an opposite spin helicity of the inner and outer Rashba bands with a different spin polarization in agreement with theoretical predictions, confirming a complex spin texture of bulk Rashba states. The outer band has about twice larger spin polarization than the inner one, giving evidence of a spin-orbit effect being related to the orbital composition of the band states. The switchable inner electric field of GeTe implies new functionalities for spintronic devices.

  5. Using arterial spin labeling to examine mood states in youth

    PubMed Central

    Mikita, Nina; Mehta, Mitul A; Zelaya, Fernando O; Stringaris, Argyris

    2015-01-01

    Introduction Little is known about the neural correlates of mood states and the specific physiological changes associated with their valence and duration, especially in young people. Arterial spin labeling (ASL) imaging is particularly well-suited to study sustained cerebral states in young people, due to its robustness to low-frequency drift, excellent interscan reliability, and noninvasiveness. Yet, it has so far been underutilized for understanding the neural mechanisms underlying mood states in youth. Methods In this exploratory study, 21 healthy adolescents aged 16 to 18 took part in a mood induction experiment. Neutral, sad, and happy mood states were induced using film clips and explicit instructions. An ASL scan was obtained following presentation of each film clip. Results Mood induction led to robust changes in self-reported mood ratings. Compared to neutral, sad mood was associated with increased regional cerebral blood flow (rCBF) in the left middle frontal gyrus and anterior prefrontal cortex, and decreased rCBF in the right middle frontal gyrus and the inferior parietal lobule. A decrease in self-reported mood from neutral to sad condition was associated with increased rCBF in the precuneus. Happy mood was associated with increased rCBF in medial frontal and cingulate gyri, the subgenual anterior cingulate cortex, and ventral striatum, and decreased rCBF in the inferior parietal lobule. The level of current self-reported depressive symptoms was negatively associated with rCBF change in the cerebellum and lingual gyrus following both sad and happy mood inductions. Conclusions Arterial spin labeling is sensitive to experimentally induced mood changes in healthy young people. The effects of happy mood on rCBF patterns were generally stronger than the effects of sad mood. PMID:26085964

  6. High-spin states with the (p,π) reaction

    NASA Astrophysics Data System (ADS)

    Jacobs, W. W.

    1986-06-01

    Data from systematic studies of the A(p,π-)A+1 reaction leading to discrete and continuous nuclear final states have revealed both expected and unexpected signatures of the dominance of a two nucleon mechanism (TNM—NN → NNπ inside the nucleus) in near-threshold pion production. A distinctive manifestation of this dominance is the systematic and selective excitation by TNM (p,π-) of high-spin 2p-1h states on target nuclei throughout the periodic table, representing a universal and fundamental response of the nucleus to this high momentum transfer probe. Questions as to whether TNM is also dominant in A(p,π+)A+1, what are the corresponding implications for high-spin excitations, and to what extent is the overall observed (p,π+) behavior related to what is known about fundamental NN → NNπ+ processes are addressed through investigation of the 13C(p,π±) reactions populating the mirror nuclei 14C and 14O. In the course of these studies, comparative (p,π+) vs. (p,π-) data were used to suggest a Jπ=5- assignment for a previously unobserved state near EX=15 MeV in the (p,π+) spectra. Also of interest is a strong and sharp (p,π+) transition at relatively high excitation (EX ≂ 23.2 MeV) in 14C. While we find most observed features in the (p,π±) spectra are consistent with TNM expectations, one possible explanation for the latter state's unique behavior involves the anomalous enhancement of normally weak free NN → NNπ isospin channels when immersed in the nuclear medium.

  7. Symmetry breaking and light-induced spin-state trapping in a mononuclear FeII complex with the two-step thermal conversion

    NASA Astrophysics Data System (ADS)

    Buron-Le Cointe, M.; Ould Moussa, N.; Trzop, E.; Moréac, A.; Molnar, G.; Toupet, L.; Bousseksou, A.; Létard, J. F.; Matouzenko, G. S.

    2010-12-01

    Crystallographic, magnetic, and Raman investigations of the mononuclear [FeII(Hpy-DAPP)](BF4)2 complex are presented. Its particular feature is a two-step thermal spin conversion in spite of a unique symmetry-independent iron site per unit cell. The plateau around 140 K is associated with a symmetry breaking visible by the appearance of weak (0k0) k odd Bragg peaks. Symmetries of the high-temperature high-spin state and of the low-temperature low-spin state are both monoclinic P21/c , so that the symmetry breaking on the plateau is associated with a reentrant phase transition. It is discussed in relation with Ising-type microscopic models. At the plateau level, the two symmetry-independent molecules differ both by their spin state and the conformation (chair versus twist-boat) of one metallocycle. At low-temperature photoinduced phenomena have been investigated: a partial phototransformation [light-induced excited spin-state trapping (LIESST) effect] is observed under visible red irradiation. Raman spectroscopy shows that the molecular photoinduced state is the high-spin one. Nevertheless, as no macroscopic symmetry breaking is observed, the unique average cationic [FeII(Hpy-DAPP)] state of the unit cell is intermediate between pure low-spin and high-spin states and presents a conformational disorder for one metallocycle. Reverse-LIESST has also been evidenced using near infrared excitation. Thus, the mononuclear [Fe(Hpy-DAPP)](BF4)2 compound offers the opportunity to discuss the interplay between spin conversion, molecular conformational change, and ordering processes.

  8. Habitability of Waterworlds: Runaway Greenhouses, Atmospheric Expansion, and Multiple Climate States of Pure Water Atmospheres

    PubMed Central

    2015-01-01

    Abstract There are four different stable climate states for pure water atmospheres, as might exist on so-called “waterworlds.” I map these as a function of solar constant for planets ranging in size from Mars-sized to 10 Earth-mass. The states are as follows: globally ice covered (Ts⪅245 K), cold and damp (270⪅Ts⪅290 K), hot and moist (350⪅Ts⪅550 K), and very hot and dry (Tsx2A86;900 K). No stable climate exists for 290⪅Ts ⪅350 K or 550⪅Ts⪅900 K. The union of hot moist and cold damp climates describes the liquid water habitable zone, the width and location of which depends on planet mass. At each solar constant, two or three different climate states are stable. This is a consequence of strong nonlinearities in both thermal emission and the net absorption of sunlight. Across the range of planet sizes, I account for the atmospheres expanding to high altitudes as they warm. The emitting and absorbing surfaces (optical depth of unity) move to high altitude, making their area larger than the planet surface, so more thermal radiation is emitted and more sunlight absorbed (the former dominates). The atmospheres of small planets expand more due to weaker gravity; the effective runaway greenhouse threshold is about 35 W m−2 higher for Mars, 10 W m−2 higher for Earth or Venus, but only a few W m−2 higher for a 10 Earth-mass planet. There is an underlying (expansion-neglected) trend of increasing runaway greenhouse threshold with planetary size (40 W m−2 higher for a 10 Earth-mass planet than for Mars). Summing these opposing trends means that Venus-sized (or slightly smaller) planets are most susceptible to a runaway greenhouse. The habitable zone for pure water atmospheres is very narrow, with an insolation range of 0.07 times the solar constant. A wider habitable zone requires background gas and greenhouse gas: N2 and CO2 on Earth, which are biologically controlled. Thus, habitability depends on inhabitance. Key Words

  9. Habitability of waterworlds: runaway greenhouses, atmospheric expansion, and multiple climate states of pure water atmospheres.

    PubMed

    Goldblatt, Colin

    2015-05-01

    There are four different stable climate states for pure water atmospheres, as might exist on so-called "waterworlds." I map these as a function of solar constant for planets ranging in size from Mars-sized to 10 Earth-mass. The states are as follows: globally ice covered (Ts ⪅ 245 K), cold and damp (270 ⪅ Ts ⪅ 290 K), hot and moist (350 ⪅ Ts ⪅ 550 K), and very hot and dry (Tsx2A86;900 K). No stable climate exists for 290 ⪅ T s ⪅ 350 K or 550 ⪅ Ts ⪅ 900 K. The union of hot moist and cold damp climates describes the liquid water habitable zone, the width and location of which depends on planet mass. At each solar constant, two or three different climate states are stable. This is a consequence of strong nonlinearities in both thermal emission and the net absorption of sunlight. Across the range of planet sizes, I account for the atmospheres expanding to high altitudes as they warm. The emitting and absorbing surfaces (optical depth of unity) move to high altitude, making their area larger than the planet surface, so more thermal radiation is emitted and more sunlight absorbed (the former dominates). The atmospheres of small planets expand more due to weaker gravity; the effective runaway greenhouse threshold is about 35 W m(-2) higher for Mars, 10 W m(-2) higher for Earth or Venus, but only a few W m(-2) higher for a 10 Earth-mass planet. There is an underlying (expansion-neglected) trend of increasing runaway greenhouse threshold with planetary size (40 W m(-2) higher for a 10 Earth-mass planet than for Mars). Summing these opposing trends means that Venus-sized (or slightly smaller) planets are most susceptible to a runaway greenhouse. The habitable zone for pure water atmospheres is very narrow, with an insolation range of 0.07 times the solar constant. A wider habitable zone requires background gas and greenhouse gas: N2 and CO2 on Earth, which are biologically controlled. Thus, habitability depends on inhabitance.

  10. Spin-polarized atomic nitrogen and the 7Sigma + u state of N2

    NASA Technical Reports Server (NTRS)

    Ferrante, R. F.; Stwalley, W. C.

    1983-01-01

    The first self-consistent field (SCF) calculation of the repulsive 7Sigma + u state of molecular nitrogen is presented. This calculation is used with attractive dispersion to provide a model potential for electron spin-polarized atomic nitrogen N appropriate in the range of 2.5-20A(O). Potential parameters obtained from the calculation are used to provide estimates of equilibrium thermodynamic properties of spin-polarized N in the quantum theorem of corresponding states framework. Consideration is given to increased stability of spin-polarized N with respect to single electron spin-flip processes, as compared to spin-polarized H.

  11. Geophysics of Titan from gravity, topography and spin state

    NASA Astrophysics Data System (ADS)

    Nimmo, F.; Bills, B. G.

    2011-12-01

    For the terrestrial planets, combined analyses of gravity and topography have greatly improved our understanding of these bodies' interiors [1]. The spin state and orientation of a planetary body can also be diagnostic of its internal structure [2]. Recently acquired topography [3], gravity [4] and spin pole constraints [5] now permit these kinds of geophysical analyses at Titan. Titan's degree-two gravity coefficients, but not those of its topography, are in the 10/3 ratio expected for a hydrostatic body. One explanation for this discrepancy is the existence of a floating isostatic ice shell whose thickness varies spatially due to tidal dissipation [6]. Shell thickness variations can result in slow non-synchronous rotation [7]. Furthermore, such variations will affect the gravity, an effect that should be taken into account when using gravity to calculate Titan's moment of inertia [4]. The relationship between the degree-three gravity and topography can be used to place constraints on the thickness and rigidity of the ice shell. Based on the inferred heat fluxes of [6], Titan's ice shell is unlikely to be less than 90% compensated at degree three. The measured degree-three gravity [4] and topography [3] coefficients show a strong correlation (r=0.84). For a completely compensated ice shell, the implied shell thickness is about 350 km, while if the shell is 90% compensated the thickness is 250 km. These shell thickness estimates significantly exceed those based on theoretical models [8,9] and surface topography [6]. One possible explanation for this discrepancy is that there are other sources of degree-three gravity (e.g. bumps on the presumed silicate core) that do not contribute significantly to the surface topography. Further gravity observations will help to resolve this issue. If a satellite's spin and orbit poles remain coplanar as the latter precesses around the invariable pole, the satellite is said to occupy a damped Cassini state and the obliquity (angle

  12. Recent Numerical Studies of the Spin Glass State

    NASA Astrophysics Data System (ADS)

    Palassini, Matteo

    2001-03-01

    The nature of the low temperature phase of spin glasses remains a controversial issue, which has recently received considerable renewed interest. Two theories have been extensively discussed: the droplet model and the replica symmetry breaking theory. In this talk, I will discuss some recent investigations of the low temperature phase of Ising spin glasses with short range interactions in three and four dimensions. I will present the results of a new approach [1] based on studying changes in the ground state when an external perturbation is applied, using efficient optimization algorithms, as well as the results of Monte Carlo simulations at very low temperatures [2]. I will compare these results with several theoretical scenarios: the droplet model, the replica symmetry breaking theory, and a new intermediate scenario in which there are large scale excitations which cost a finite energy in the thermodynamic limit, but whose surface has a vanishing density. [1] M.Palassini and A.P. Young, Phys. Rev. Lett. 85, 3017 (2000); Phys. Rev. Lett. 83, 5126 (1999); and unpublished. [2] H.G. Katzgraber, M.Palassini and A.P. Young, cond-mat/0007113; M.Palassini and A.P.Young, unpublished.

  13. Externally controlled spin state switching in metal-organic complexes.

    NASA Astrophysics Data System (ADS)

    Bagrets, Alexei; Meded, Velimir; Ruben, Mario; Evers, Ferdinand

    2009-03-01

    Recent transport experiments have demonstrated that a manipulation of the charge of individual molecules is feasible using electromigrated metal junctions [1] or electrochemical gates in conjunction with the STM [2]. Using elaborated density functional theory calculations, we will discuss a possibility to induce -- by means of charging or applied stress -- a switching between low and high spin states in certain metal-organic systems, [Fe(bpp)2]^2+ (bpp: bispyrazolyl pyridine) and [Mn(tpy)2]^2+ (tpy: terpyridine). Based upon a recent success of the single molecular conduction experiment through Ru(II) complex [3], we anticipate the transport properties of Fe(II) and Mn(II) complexes to be gate controlled via exploiting their spin degree of freedom. [1] E. A. Osorio et al., J. Phys.: Condens. Matter20, 374121 (2008); [2] F. Chen el al., Ann. Rev. Phys. Chem. 58, 535 (2007); Li et al., Nanotechnology 18, 044018 (2007). [3] M. Ruben, A. Landa, E. L"ortscher, H. Riel, M. Mayor, H. G"orls, H. Weber, A. Arnold, and F. Evers, Small (online), DOI: 10.1002/smll.200800390 (2008).

  14. Ground-state energies of the nonlinear sigma model and the Heisenberg spin chains

    NASA Technical Reports Server (NTRS)

    Zhang, Shoucheng; Schulz, H. J.; Ziman, Timothy

    1989-01-01

    A theorem on the O(3) nonlinear sigma model with the topological theta term is proved, which states that the ground-state energy at theta = pi is always higher than the ground-state energy at theta = 0, for the same value of the coupling constant g. Provided that the nonlinear sigma model gives the correct description for the Heisenberg spin chains in the large-s limit, this theorem makes a definite prediction relating the ground-state energies of the half-integer and the integer spin chains. The ground-state energies obtained from the exact Bethe ansatz solution for the spin-1/2 chain and the numerical diagonalization on the spin-1, spin-3/2, and spin-2 chains support this prediction.

  15. Ground-state energies of the nonlinear sigma model and the Heisenberg spin chains

    NASA Technical Reports Server (NTRS)

    Zhang, Shoucheng; Schulz, H. J.; Ziman, Timothy

    1989-01-01

    A theorem on the O(3) nonlinear sigma model with the topological theta term is proved, which states that the ground-state energy at theta = pi is always higher than the ground-state energy at theta = 0, for the same value of the coupling constant g. Provided that the nonlinear sigma model gives the correct description for the Heisenberg spin chains in the large-s limit, this theorem makes a definite prediction relating the ground-state energies of the half-integer and the integer spin chains. The ground-state energies obtained from the exact Bethe ansatz solution for the spin-1/2 chain and the numerical diagonalization on the spin-1, spin-3/2, and spin-2 chains support this prediction.

  16. Electric field controlled spin- and valley-polarized edge states in silicene with extrinsic Rashba effect

    NASA Astrophysics Data System (ADS)

    Yu, Zhiming; Pan, Hui; Yao, Yugui

    2015-10-01

    In the presence of extrinsic Rashba spin-orbit coupling, we find that silicene can host a quantum anomalous Hall state with spin- and valley-polarized edge states, which can be effectively controlled by the exchange field and electric field. In this state, a pair of nontrivial edge states reside in one specific valley and have a strong but opposite spin polarization. A distinctive feature of this state is that both of the spin and valley indexes of the edge states can be switched by reversing the electric field. We also present a microscopic mechanism for the origin of this state. Our findings provide an efficient way to control the topologically protected spin- and valley-polarized edge states, which is crucial for spintronics and valleytronics.

  17. Spin State as a Marker for the Structural Evolution of Nature's Water-Splitting Catalyst.

    PubMed

    Krewald, Vera; Retegan, Marius; Neese, Frank; Lubitz, Wolfgang; Pantazis, Dimitrios A; Cox, Nicholas

    2016-01-19

    In transition-metal complexes, the geometric structure is intimately connected with the spin state arising from magnetic coupling between the paramagnetic ions. The tetramanganese-calcium cofactor that catalyzes biological water oxidation in photosystem II cycles through five catalytic intermediates, each of which adopts a specific geometric and electronic structure and is thus characterized by a specific spin state. Here, we review spin-structure correlations in Nature's water-splitting catalyst. The catalytic cycle of the Mn4O5Ca cofactor can be described in terms of spin-dependent reactivity. The lower "inactive" S states of the catalyst, S0 and S1, are characterized by low-spin ground states, SGS = 1/2 and SGS = 0. This is connected to the "open cubane" topology of the inorganic core in these states. The S2 state exhibits structural and spin heterogeneity in the form of two interconvertible isomers and is identified as the spin-switching point of the catalytic cycle. The first S2 state form is an open cubane structure with a low-spin SGS = 1/2 ground state, whereas the other represents the first appearance of a closed cubane topology in the catalytic cycle that is associated with a higher-spin ground state of SGS = 5/2. It is only this higher-spin form of the S2 state that progresses to the "activated" S3 state of the catalyst. The structure of this final metastable catalytic state was resolved in a recent report, showing that all manganese ions are six-coordinate. The magnetic coupling is dominantly ferromagnetic, leading to a high-spin ground state of SGS = 3. The ability of the Mn4O5Ca cofactor to adopt two distinct structural and spin-state forms in the S2 state is critical for water binding in the S3 state, allowing spin-state crossing from the inactive, low-spin configuration of the catalyst to the activated, high-spin configuration. Here we describe how an understanding of the magnetic properties of the catalyst in all S states has allowed conclusions on

  18. Pure absorption electron spin echo envelope modulation spectra by using the filter-diagonalization method for harmonic inversion.

    PubMed

    Jeschke, G; Mandelshtam, V A; Shaka, A J

    1999-03-01

    Harmonic inversion of electron spin echo envelope (ESEEM) time-domain signals by filter diagonalization is investigated as an alternative to Fourier transformation. It is demonstrated that this method features enhanced resolution compared to Fourier-transform magnitude spectra, since it can eliminate dispersive contributions to the line shape, even if no linear phase correction is possible. Furthermore, instrumental artifacts can be easily removed from the spectra if they are narrow either in time or frequency domain. This applies to echo crossings that are only incompletely eliminated by phase cycling and to spurious spectrometer frequencies, respectively. The method is computationally efficient and numerically stable and does not require extensive parameter adjustments or advance knowledge of the number of spectral lines. Experiments on gamma-irradiated methyl-alpha-d-glucopyranoside show that more information can be obtained from typical ESEEM time-domain signals by filter-diagonalization than by Fourier transformation.

  19. Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet.

    PubMed

    Han, Tian-Heng; Helton, Joel S; Chu, Shaoyan; Nocera, Daniel G; Rodriguez-Rivera, Jose A; Broholm, Collin; Lee, Young S

    2012-12-20

    The experimental realization of quantum spin liquids is a long-sought goal in physics, as they represent new states of matter. Quantum spin liquids cannot be described by the broken symmetries associated with conventional ground states. In fact, the interacting magnetic moments in these systems do not order, but are highly entangled with one another over long ranges. Spin liquids have a prominent role in theories describing high-transition-temperature superconductors, and the topological properties of these states may have applications in quantum information. A key feature of spin liquids is that they support exotic spin excitations carrying fractional quantum numbers. However, detailed measurements of these 'fractionalized excitations' have been lacking. Here we report neutron scattering measurements on single-crystal samples of the spin-1/2 kagome-lattice antiferromagnet ZnCu(3)(OD)(6)Cl(2) (also called herbertsmithite), which provide striking evidence for this characteristic feature of spin liquids. At low temperatures, we find that the spin excitations form a continuum, in contrast to the conventional spin waves expected in ordered antiferromagnets. The observation of such a continuum is noteworthy because, so far, this signature of fractional spin excitations has been observed only in one-dimensional systems. The results also serve as a hallmark of the quantum spin-liquid state in herbertsmithite.

  20. Transferring entangled states through spin chains by boundary-state multiplets

    NASA Astrophysics Data System (ADS)

    Lorenz, Peter; Stolze, Joachim

    2014-10-01

    Quantum spin chains may be used to transfer quantum states between elements of a quantum information processing device. A scheme discovered recently [Phys. Rev. A 85, 022312 (2012), 10.1103/PhysRevA.85.022312] was shown to have favorable transfer properties for single-qubit states even in the presence of built-in static disorder caused by manufacturing errors. We extend that scheme in a way suggested already in Bruderer et al. [Phys. Rev. A 85, 022312 (2012), 10.1103/PhysRevA.85.022312] and study the transfer of the four Bell states which form a maximally entangled basis in the two-qubit Hilbert space. We show that perfect transfer of all four Bell states separately and of arbitrary linear combinations may be achieved for chains with hundreds of spins. For simplicity we restrict ourselves to systems without disorder.

  1. Theoretical study of dynamic electron-spin-polarization via the doublet-quartet quantum-mixed state and time-resolved ESR spectra of the quartet high-spin state.

    PubMed

    Teki, Yoshio; Matsumoto, Takafumi

    2011-04-07

    The mechanism of the unique dynamic electron polarization of the quartet (S = 3/2) high-spin state via a doublet-quartet quantum-mixed state and detail theoretical calculations of the population transfer are reported. By the photo-induced electron transfer, the quantum-mixed charge-separate state is generated in acceptor-donor-radical triad (A-D-R). This mechanism explains well the unique dynamic electron polarization of the quartet state of A-D-R. The generation of the selectively populated quantum-mixed state and its transfer to the strongly coupled pure quartet and doublet states have been treated both by a perturbation approach and by exact numerical calculations. The analytical solutions show that generation of the quantum-mixed states with the selective populations after de-coherence and/or accompanying the (complete) dephasing during the charge-recombination are essential for the unique dynamic electron polarization. Thus, the elimination of the quantum coherence (loss of the quantum information) is the key process for the population transfer from the quantum-mixed state to the quartet state. The generation of high-field polarization on the strongly coupled quartet state by the charge-recombination process can be explained by a polarization transfer from the quantum-mixed charge-separate state. Typical time-resolved ESR patterns of the quantum-mixed state and of the strongly coupled quartet state are simulated based on the generation mechanism of the dynamic electron polarization. The dependence of the spectral pattern of the quartet high-spin state has been clarified for the fine-structure tensor and the exchange interaction of the quantum-mixed state. The spectral pattern of the quartet state is not sensitive towards the fine-structure tensor of the quantum-mixed state, because this tensor contributes only as a perturbation in the population transfer to the spin-sublevels of the quartet state. Based on the stochastic Liouville equation, it is also

  2. Laser induced spin state transition: Spectral and temporal evolution

    NASA Astrophysics Data System (ADS)

    Fouché, O.; Degert, J.; Jonusauskas, G.; Baldé, C.; Desplanche, C.; Létard, J. F.; Freysz, E.

    2009-02-01

    At 150 K, we have recorded the evolution of the energy threshold versus the wavelength and the kinetic of formation and relaxation of the spin state phase transition induced by a single laser pulse in the [Fe(PM-BiA)2(NCS)2] compound. We demonstrate that different absorption bands of the complexes can drive the phase transition. The saturation-energy and the threshold-energy of the laser pulses are not directly related to the absorption cross-section of the sample. Both the switching and the relaxation kinetics are well fitted using two different time-constants. The switching lasts about 50 μs. The relaxation time-constants are independent of the used excitation-wavelength.

  3. Color spin wave functions of heavy tetraquark states

    NASA Astrophysics Data System (ADS)

    Park, Woosung; Lee, Su Houng

    2014-05-01

    Using the variational method, we calculate the mass of the JP=1+udbbarbbar tetraquark containing two identical heavy antiquarks in a nonrelativistic potential model with color confinement and spin hyperfine interaction. In particular, we extend a previous investigation of the model by Brink and Stancu by investigating the effect of including the color anti-sextet component of the diquark configuration as well as using several more Gaussian parametrization for the L=0 part of the spatial wave function. We find that for the heavy tetraquark, the 66bar component among the color singlet bases is negligible and that the previously used specific Gaussian spatial configuration is good enough in obtaining the ground state energy.

  4. Thermal Equilibrium of a Macroscopic Quantum System in a Pure State

    NASA Astrophysics Data System (ADS)

    Goldstein, Sheldon; Huse, David A.; Lebowitz, Joel L.; Tumulka, Roderich

    2015-09-01

    We consider the notion of thermal equilibrium for an individual closed macroscopic quantum system in a pure state, i.e., described by a wave function. The macroscopic properties in thermal equilibrium of such a system, determined by its wave function, must be the same as those obtained from thermodynamics, e.g., spatial uniformity of temperature and chemical potential. When this is true we say that the system is in macroscopic thermal equilibrium (MATE). Such a system may, however, not be in microscopic thermal equilibrium (MITE). The latter requires that the reduced density matrices of small subsystems be close to those obtained from the microcanonical, equivalently the canonical, ensemble for the whole system. The distinction between MITE and MATE is particularly relevant for systems with many-body localization for which the energy eigenfuctions fail to be in MITE while necessarily most of them, but not all, are in MATE. We note, however, that for generic macroscopic systems, including those with MBL, most wave functions in an energy shell are in both MATE and MITE. For a classical macroscopic system, MATE holds for most phase points on the energy surface, but MITE fails to hold for any phase point.

  5. Time-Domain Pure-state Polarization Analysis of Surface Waves Traversing California

    SciTech Connect

    Zhang, J; Walter, W R; Lay, T; Wu, R

    2003-11-04

    A time-domain pure-state polarization analysis method is used to characterize surface waves traversing California parallel to the plate boundary. The method is applied to data recorded at four broadband stations in California from twenty-six large, shallow earthquakes which occurred since 1988, yielding polarization parameters such as the ellipticity, Euler angles, instantaneous periods, and wave incident azimuths. The earthquakes are located along the circum-Pacific margin and the ray paths cluster into two groups, with great-circle paths connecting stations MHC and PAS or CMB and GSC. The first path (MHC-PAS) is in the vicinity of the San Andreas Fault System (SAFS), and the second (CMB-GSC) traverses the Sierra Nevada Batholith parallel to and east of the SAFS. Both Rayleigh and Love wave data show refractions due to lateral velocity heterogeneities under the path, indicating that accurate phase velocity and attenuation analysis requires array measurements. The Rayleigh waves are strongly affected by low velocity anomalies beneath Central California, with ray paths bending eastward as waves travel toward the south, while Love waves are less affected, providing observables to constrain the depth extent of the anomalies. Strong lateral gradients in the lithospheric structure between the continent and the ocean are the likely cause of the path deflections.

  6. Thermal Equilibrium of a Macroscopic Quantum System in a Pure State.

    PubMed

    Goldstein, Sheldon; Huse, David A; Lebowitz, Joel L; Tumulka, Roderich

    2015-09-04

    We consider the notion of thermal equilibrium for an individual closed macroscopic quantum system in a pure state, i.e., described by a wave function. The macroscopic properties in thermal equilibrium of such a system, determined by its wave function, must be the same as those obtained from thermodynamics, e.g., spatial uniformity of temperature and chemical potential. When this is true we say that the system is in macroscopic thermal equilibrium (MATE). Such a system may, however, not be in microscopic thermal equilibrium (MITE). The latter requires that the reduced density matrices of small subsystems be close to those obtained from the microcanonical, equivalently the canonical, ensemble for the whole system. The distinction between MITE and MATE is particularly relevant for systems with many-body localization for which the energy eigenfuctions fail to be in MITE while necessarily most of them, but not all, are in MATE. We note, however, that for generic macroscopic systems, including those with MBL, most wave functions in an energy shell are in both MATE and MITE. For a classical macroscopic system, MATE holds for most phase points on the energy surface, but MITE fails to hold for any phase point.

  7. A four-parameter corresponding-states method for prediction of Newtonian, pure-component viscosity

    NASA Astrophysics Data System (ADS)

    Okeson, K. J.; Rowley, R. L.

    1991-01-01

    The extended Lee-Kesler (ELK) method, introduced for calculating thermodynamic properties of polar as well as nonpolar fluids and their mixtures, has been adapted to the calculation of Newtonian, pure-fluid viscosity. The method is a four-parameter, corresponding-states technique requiring as input the critical temperature, critical pressure, a size/shape parameter α, and a polar interaction parameter β. Because α and β have been previously tabulated for many fluids (for calculation of thermodynamic properties) and may also be obtained directly from the radius of gyration and a single liquid density, respectively, the method contains no adjustable parameters and is predictive in nature. ELK viscosity predictions were compared to experimental data for nonpolar and polar fluids. For 36 different nonpolar fluids and a total of 5748 different points, the comparison yielded an absolute average deviation (AAD) of 7.88% with a bias of -4.45%. Similarly, the AAD was 10.62% with a bias of -5.34% for a comparison of 15 different polar fluids involving 1500 different points. With this method, viscosities can be calculated within the range 0.55 ⩽ T r⩽2.00 and 0< P r⩽10.

  8. Spin eigen-states of Dirac equation for quasi-two-dimensional electrons

    SciTech Connect

    Eremko, Alexander; Brizhik, Larissa; Loktev, Vadim

    2015-10-15

    Dirac equation for electrons in a potential created by quantum well is solved and the three sets of the eigen-functions are obtained. In each set the wavefunction is at the same time the eigen-function of one of the three spin operators, which do not commute with each other, but do commute with the Dirac Hamiltonian. This means that the eigen-functions of Dirac equation describe three independent spin eigen-states. The energy spectrum of electrons confined by the rectangular quantum well is calculated for each of these spin states at the values of energies relevant for solid state physics. It is shown that the standard Rashba spin splitting takes place in one of such states only. In another one, 2D electron subbands remain spin degenerate, and for the third one the spin splitting is anisotropic for different directions of 2D wave vector.

  9. Deformed Fredkin spin chain with extensive entanglement

    NASA Astrophysics Data System (ADS)

    Salberger, Olof; Udagawa, Takuma; Zhang, Zhao; Katsura, Hosho; Klich, Israel; Korepin, Vladimir

    2017-06-01

    We introduce a new spin chain which is a deformation of the Fredkin spin chain and has a phase transition between bounded and extensive entanglement entropy scaling. In this chain, spins have a local interaction of three nearest neighbors. The Hamiltonian is frustration-free and its ground state can be described analytically as a weighted superposition of Dyck paths that depends on a deformation parameter t. In the purely spin 1/2 case, whenever t\

  10. Pure water injection into porous rock with superheated steam and salt in a solid state

    NASA Astrophysics Data System (ADS)

    Montegrossi, G.; Tsypkin, G.; Calore, C.

    2012-04-01

    Most of geothermal fields require injection of fluid into the hot rock to maintain pressure and productivity. The presence of solid salt in porous space may cause an unexpected change in the characteristics of the reservoir and produced fluids, and dramatically affect the profitability of the project. We consider an injection problem of pure water into high temperature geothermal reservoir, saturated with superheated vapour and solid salt. Pure water moves away from injection point and dissolves solid salt. When salty water reaches the low-pressure hot domain, water evaporation occurs and, consequently, salt precipitates. We develop a simplified analytical model of the process and derive the similarity solutions for a 1-D semi-infinite reservoir. These solutions are multi-valued and describe the reduction in permeability and porosity due to salt precipitation at the leading boiling front. If the parameters of the system exceed critical values, then similarity solution ceases to exist. We identify this mathematical behaviour with reservoir sealing in the physical system. The TOUGH2-EWASG code has been used to verify this hypothesis and investigate the precipitate formation for an idealized bounded 1-D geothermal system of a length of 500 m with water injection at one extreme and fluid extraction at the other one. Both boundaries are kept at constant pressure and temperature. The result for the semi-infinite numerical model show that the monotonic grow of the solid salt saturation to reach asymptotic similarity solution generally occurs over a very large length starting from the injection point. Reservoir sealing occurs if solid salt at the initial state occupies a considerable part of the porous space. Numerical experiments for the bounded 500 m system demonstrate that a small amount of salt is enough to get reservoir sealing. Generally, salt tend to accumulate near the production well, and salt plug forms at the elements adjacent to the extraction point. This type

  11. Electronic states and spin-orbit splitting of lanthanum dimer

    NASA Astrophysics Data System (ADS)

    Liu, Yang; Wu, Lu; Zhang, Chang-Hua; Krasnokutski, Serge A.; Yang, Dong-Sheng

    2011-07-01

    Lanthanum dimer (La2) was studied by mass-analyzed threshold ionization (MATI) spectroscopy and a series of multi-configuration ab initio calculations. The MATI spectrum exhibits three band systems originating from ionization of the neutral ground electronic state, and each system shows vibrational frequencies of the neutral molecule and singly charged cation. The three ionization processes are La2+ (a2∑g+) ← La2 (X1∑g+), La2+ (b2Π3/2, u) ← La2 (X1∑g+), and La2+ (b2Π1/2, u) ← La2 (X1∑g+), with the ionization energies of 39 046, 40 314, and 40 864 cm-1, respectively. The vibrational frequency of the X1Σg+ state is 207 cm-1, and those of the a2Σg+, b2Π3/2, u and b2Π1/2, u are 235.7, 242.2, and 240 cm-1. While X1Σg+ is the ground state of the neutral molecule, a2Σg+ and b2Πu are calculated to be the excited states of the cation. The spin-orbit splitting in the b2Πu ion is 550 cm-1. An X4Σg- state of La2+ was predicted by theory, but not observed by the experiment. The determination of a singlet ground state of La2 shows that lanthanum behaves differently from scandium and yttrium.

  12. Spin state transition in the active center of the hemoglobin molecule: DFT + DMFT study

    NASA Astrophysics Data System (ADS)

    Novoselov, D.; Korotin, Dm. M.; Anisimov, V. I.

    2016-05-01

    An ab initio study of electronic and spin configurations of the iron ion in the active center of the human hemoglobin molecule is presented. With a combination of the Density Functional Theory (DFT) method and the Dynamical Mean Field Theory (DMFT) approach, the spin state transition description in the iron ion during the oxidation process is significantly improved in comparison with previous attempts. It was found that the origin of the iron ion local moment behavior both for the high-spin and for the low-spin states in the hemoglobin molecule is caused by the presence of a mixture of several atomic states with comparable statistical probability.

  13. Spin-spiral states in undoped manganites: role of finite Hund's rule coupling.

    PubMed

    Kumar, Sanjeev; van den Brink, Jeroen; Kampf, Arno P

    2010-01-08

    The experimental observation of multiferroic behavior in perovskite manganites with a spiral spin structure requires a clarification of the origin of these magnetic states and their relation to ferroelectricity. We show that spin-spiral phases with a diagonal wave vector and also an E-type phase exist for intermediate value of Hund's rule and the Jahn-Teller coupling in the orbitally ordered and insulating state of the standard two-band model Hamiltonian for manganites. Our results support the spin-current mechanism for ferroelectricity and present an alternative view to earlier conclusions where frustrating superexchange couplings were crucial to obtaining spin-spiral states.

  14. Spin polarized bound states in the continuum in open Aharonov-Bohm rings with the Rashba spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Bulgakov, Evgeny N.; Sadreev, Almas F.

    2016-07-01

    We consider the trapping of electrons with a definite spin polarization by bound states in the continuum (BSC) in the open Aharonov-Bohm rings in the presence of the Rashba spin-orbit interaction (RSOI). Neglecting the Zeeman term we show the existence of BSCs in the one-dimensional ring when the eigenstates of the closed ring are doubly degenerate. With account of the Zeeman term BSCs occur only at the points of threefold degeneracy. The BSCs are found in the parametric space of flux and RSOI strength in close pairs with opposite spin polarization. Thereby the spin polarization of electrons transmitted through the ring can be altered by minor variation of magnetic or electric field at the vicinity of these pairs. Numerical simulations of the two-dimensional open ring show similar results for the BSCs. Encircling the BSC points in the parametric space of the flux and the RSOI constant gives rise to a geometric phase.

  15. Notes on Ground-State Properties of Mixed Spin-1 and Spin-1/2 Lieb-Lattice Heisenberg Antiferromagnets

    NASA Astrophysics Data System (ADS)

    Hirose, Yuhei; Miura, Shoma; Yasuda, Chitoshi; Fukumoto, Yoshiyuki

    2017-08-01

    Quantum Monte Carlo (QMC) simulations are performed to study ground-state properties of a mixed spin-1 and spin-1/2 Lieb-lattice Heisenberg antiferromagnet, in order to get further insight beyond the modified spin-wave (MSW) study reported in [J. Phys. Soc. Jpn. 86, 014002 (2017)]. It is confirmed that the MSW results are in good agreement with the QMC results. In particular, the scaling relation found in the MSW study, which argues that sublattice spin reductions are inversely proportional to the sublattice sizes, is observed in our QMC simulation. We present a rigorous proof for spontaneous sublattice magnetizations induced by an infinitesimal uniform magnetic field. The calculation process in the MSW theory is reexamined to clarify the mathematical structure behind the scaling relation for sublattice long-range orders.

  16. Spin polarized bound states in the continuum in open Aharonov-Bohm rings with the Rashba spin-orbit interaction.

    PubMed

    Bulgakov, Evgeny N; Sadreev, Almas F

    2016-07-06

    We consider the trapping of electrons with a definite spin polarization by bound states in the continuum (BSC) in the open Aharonov-Bohm rings in the presence of the Rashba spin-orbit interaction (RSOI). Neglecting the Zeeman term we show the existence of BSCs in the one-dimensional ring when the eigenstates of the closed ring are doubly degenerate. With account of the Zeeman term BSCs occur only at the points of threefold degeneracy. The BSCs are found in the parametric space of flux and RSOI strength in close pairs with opposite spin polarization. Thereby the spin polarization of electrons transmitted through the ring can be altered by minor variation of magnetic or electric field at the vicinity of these pairs. Numerical simulations of the two-dimensional open ring show similar results for the BSCs. Encircling the BSC points in the parametric space of the flux and the RSOI constant gives rise to a geometric phase.

  17. Spin-wave singularities: Free energy and equation of state in O(n) spin models near Tc

    NASA Astrophysics Data System (ADS)

    Weichman, Peter B.; Kim, Kihong

    1990-12-01

    We give a detailed derivation of the thermodynamics of O(n) spin models, correct to O(ɛ=4-d), using a generalization of the renormalization-group trajectory integral and noncritical matching technique first introduced by Rudnick and Nelson. The results are valid throughout the critical region, both with and without external magnetic field. We especially emphasize the coexistence-curve behavior for spins with a continuous symmetry (n>=2), deriving detailed expressions for the renormalized spin-wave stiffness (superfluid density) and longitudinal susceptibility. We generalize the parametric representation for the equation of state to include spin-wave singularities, yielding corrections to the so-called ``linear model.'' Our expression for the free energy differs in some details from that given previously by Nicoll and Chang, necessitating minor corrections to previous applications to the weakly interacting Bose gas at constant density.

  18. Pseudoentanglement of Spin States in the Multilevel 15N@C60 System

    NASA Astrophysics Data System (ADS)

    Mehring, M.; Scherer, W.; Weidinger, A.

    2004-11-01

    We have prepared combined electron and nuclear spin pseudoentangled states Ψ±27 and Φ±18 out of the total number of eight quantum states in the multilevel quantum system of a nitrogen atom with electron spin 3/2 and nuclear spin 1/2 encaged in the endohedral fullerene 15N@C60. Density matrix tomography was applied to verify the degree of entanglement.

  19. High-sensitivity single NV magnetometry by spin-to-charge state mapping

    NASA Astrophysics Data System (ADS)

    Jaskula, Jean-Christophe; Shields, Brendan; Bauch, Erik; Lukin, Mikhail; Walsworth, Ronald; Trifonov, Alexei

    2015-05-01

    Nitrogen-Vacancy (NV) centers in diamond are atom-like quantum system in a solid state matrix whom its structure allows optical readout of the electronic spin. However, the optimal duration of optical readout is limited by a singlet state lifetime making single shot spin readout out of reach. On the other side, the NV center charge state readout can be extremely efficient (up to 99% fidelity) by using excitation at 594 nm. We will present a new method of spin readout utilizing a spin-depending photoionization process to map the electronic spin state of the NV onto the its charge state. Moreover, pre-selection on the charged state allows to minimize data acquisition time. This scheme improves single NV AC magnetometry by a factor of 5 and will benefit other single NV center experiments as well.

  20. Theory of inelastic neutron scattering in a field-induced spin-nematic state

    NASA Astrophysics Data System (ADS)

    Smerald, Andrew; Ueda, Hiroaki T.; Shannon, Nic

    2015-05-01

    We develop a theory of spin excitations in a field-induced spin-nematic state, and use it to show how a spin-nematic order can be indentified using inelastic neutron scattering. We concentrate on two-dimensional frustrated ferromagnets, for which a two-sublattice, bond-centered spin-nematic state is predicted to exist over a wide range of parameters. First, to clarify the nature of spin-excitations, we introduce a soluble spin-1 model, and use this to derive a continuum field theory, applicable to any two-sublattice spin-nematic state. We then parameterize this field theory, using diagrammatic calculations for a realistic microscopic model of a spin-1/2 frustrated ferromagnet, and show how it can be used to make predictions for inelastic neutron scattering. As an example, we show quantitative predictions for inelastic scattering of neutrons from BaCdVO(PO 4)2 , a promising candidate to realize a spin-nematic state at an achievable h ˜4 T. We show that in this material it is realistic to expect a ghostly Goldstone mode, signalling spin-nematic order, to be visible in experiment.

  1. Hyperfine and Spin-Orbit Coupling Effects on Decay of Spin-Valley States in a Carbon Nanotube.

    PubMed

    Pei, T; Pályi, A; Mergenthaler, M; Ares, N; Mavalankar, A; Warner, J H; Briggs, G A D; Laird, E A

    2017-04-28

    The decay of spin-valley states is studied in a suspended carbon nanotube double quantum dot via the leakage current in Pauli blockade and via dephasing and decoherence of a qubit. From the magnetic field dependence of the leakage current, hyperfine and spin-orbit contributions to relaxation from blocked to unblocked states are identified and explained quantitatively by means of a simple model. The observed qubit dephasing rate is consistent with the hyperfine coupling strength extracted from this model and inconsistent with dephasing from charge noise. However, the qubit coherence time, although longer than previously achieved, is probably still limited by charge noise in the device.

  2. Hyperfine and Spin-Orbit Coupling Effects on Decay of Spin-Valley States in a Carbon Nanotube

    NASA Astrophysics Data System (ADS)

    Pei, T.; Pályi, A.; Mergenthaler, M.; Ares, N.; Mavalankar, A.; Warner, J. H.; Briggs, G. A. D.; Laird, E. A.

    2017-04-01

    The decay of spin-valley states is studied in a suspended carbon nanotube double quantum dot via the leakage current in Pauli blockade and via dephasing and decoherence of a qubit. From the magnetic field dependence of the leakage current, hyperfine and spin-orbit contributions to relaxation from blocked to unblocked states are identified and explained quantitatively by means of a simple model. The observed qubit dephasing rate is consistent with the hyperfine coupling strength extracted from this model and inconsistent with dephasing from charge noise. However, the qubit coherence time, although longer than previously achieved, is probably still limited by charge noise in the device.

  3. Early stage spin-state transition in LaCoO3 investigated by first principles

    NASA Astrophysics Data System (ADS)

    Leighton, C.; Hsu, H.; Cococcioni, M.; Wentzcovitch, R. M.

    2009-12-01

    Thermal-induced spin-state transition in LaCoO3 has been a highly debated phenomenon. The point in controversy is whether the intermediate-spin (IS) state can stably exist, and whether the intermediate-spin or high-spin (HS) state is the first excited state. In our calculation, we have successfully stabilized isolated HS and IS Co in an array of low-spin (LS) Co in LaCoO3 using the local density approximation + Hubbard U (LDA+U) method. The HS/LS (or IS/LS) Co population ratio is set to 1:7, so that the early stage of spin-state transition is properly approximated. The Hubbard U is self-consistently determined by first principles, so that the equation of state and the energy of Co in each spin state can be determined with better accuracy. We show that at low temperature, isolated IS Co has higher energy than isolated HS Co. We also show that low concentration of isolated IS Co can lead to metallic LaCoO3. Therefore, the early stage spin-state transition in LaCoO3 is LS-to-HS transition. This work was supported primarily by the MRSEC Program of the National Science Foundation under Award Number DMR-0212302 and DMR-0819885. It was also partially supported by NSF grants ITR-0426757 (VLab) and EAR 0757903. Calculations were performed at Minnesota Supercomputing Institute (MSI).

  4. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet

    DOE PAGES

    Fu, Mingxuan; Imai, Takahashi; Han, Tian -Heng; ...

    2015-11-06

    Here, the kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χkagome, deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with themore » magnetic field dependence of χkagome that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.« less

  5. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet

    SciTech Connect

    Fu, M.; Imai, T.; Han, T. -H.; Lee, Y. S.

    2015-11-05

    The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum.We demonstrated that the intrinsic local spin susceptibility ckagome, deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of ckagome that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.

  6. NMR Search for the Spin Nematic State in LaFeAsO Single Crystal

    NASA Astrophysics Data System (ADS)

    Fu, Mingxuan; Torchetti, David A.; Imai, Takashi; Ning, Fanlong; Yan, Jiaqian; Sefat, Athena S.

    2013-03-01

    The mechanism underlying high-Tc superconductivity in iron-pnictides remains a major puzzle in condensed matter. Earlier NMR measurements provide evidence for a correlation between Tc and the enhancement of low frequency spin fluctuations[1]. However, slowing of spin fluctuations is accompanied by lattice softening, which is a major complication in this scenario. The intermediate temperature range between the tetragonal-orthorhombic structural phase transition at TTO and SDW transition at TSDW may be a realization of spin nematic state[2]. We report 75As single crystal NMR study of LaFeAsO [3]. We have found that the low frequency spin dynamics exhibits a strong two-fold anisotropy within each orthorhombic domain below TTO This intermediate state then freezes progressively into a static SDW below TSDW. Our results reveal the presence of an exotic intermediate spin state below TTO with the signature of spin nematicity.

  7. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet.

    PubMed

    Fu, Mingxuan; Imai, Takashi; Han, Tian-Heng; Lee, Young S

    2015-11-06

    The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χ(kagome), deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χ(kagome) that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.

  8. Spin polarized electronic states and spin textures at the surface of oxygen-deficient SrTiO3

    NASA Astrophysics Data System (ADS)

    Jeschke, Harald O.; Altmeyer, Michaela; Rozenberg, Marcelo; Gabay, Marc; Valenti, Roser

    We investigate the electronic structure and spin texture at the (001) surface of SrTiO3 in the presence of oxygen vacancies by means of ab initio density functional theory (DFT) calculations of slabs. Relativistic non-magnetic DFT calculations exhibit Rashba-like spin winding with a characteristic energy scale ~ 10 meV. However, when surface magnetism on the Ti ions is included, bands become spin-split with an energy difference ~ 100 meV at the Γ point. This energy scale is comparable to the observations in SARPES experiments performed on the two-dimensional electronic states confined near the (001) surface of SrTiO3. We find the spin polarized state to be the ground state of the system, and while magnetism tends to suppress the effects of the relativistic Rashba interaction, signatures of it are still clearly visible in terms of complex spin textures. We gratefully acknowledge financial support from the Deutsche Forschungsgemeinschaft through grants SFB/TR 49 and FOR 1346.

  9. Observations of high spin states in {sup 179}Au

    SciTech Connect

    Carpenter, M.P.; Ahmad, I.; Blumenthal, D.J.

    1995-08-01

    As part of a current study on the properties of the {pi} i{sub 13/2} intruder state in the A = 175-190 region, we conducted an experiment at ATLAS to observe high spin states in {sup 179}Au utilizing the reaction {sup 144}Sm({sup 40}Ar,p4n) at beam energies of 207 MeV and 215 MeV. To aid in the identification of {sup 179}Au, and to filter out the large amount of events from fission by-products, the Fragment Mass Analyzer was utilized in conjunction with ten Compton-suppression germanium detectors. In total, 11 x 10{sup 6} {gamma}-{gamma} and 4 x 10{sup 5} {gamma}-recoil events were collected. By comparing {gamma}-rays in coincidence with an A = 179 recoil mass gate and {gamma}-rays in coincidence with Au K{alpha} and K{beta} X-rays, ten {gamma}-rays were identified as belonging to {sup 179}Au. Based on {gamma}-ray coincidence relationships and on comparisons with neighboring odd-A Au nuclei, we constructed a tentative level scheme and assigned a rotational-like sequence to the {pi} i{sub 13/2} proton configuration.

  10. Memory-built-in quantum cloning in a hybrid solid-state spin register.

    PubMed

    Wang, W-B; Zu, C; He, L; Zhang, W-G; Duan, L-M

    2015-07-16

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science.

  11. Irreversible transitions in the exchange-striction model of spin-glass state

    NASA Astrophysics Data System (ADS)

    Valkov, V. I.; Golovchan, A. V.

    2014-08-01

    Based on the assumption of a negative volume dependence of random exchange integrals, it is possible to switch to a compressible Sherrington-Kirkpatrick spin-glass model. Within the proposed model, temperature-pressure phase diagrams were calculated and pressure- and magnetic-field-induced first-order phase transitions from the initial paramagnetic and spin-glass states to the ferromagnetic state were predicted. It was shown that the application of pressure in the spin-glass state not only increases and shifts magnetic susceptibility, but also reduces the critical magnetic fields of irreversible induced phase transitions from the spin-glass to the ferromagnetic state. The obtained results are used to describe the spin-glass state in (Sm1-xGdx)0.55Sr0.45MnO3.

  12. Memory-built-in quantum cloning in a hybrid solid-state spin register

    NASA Astrophysics Data System (ADS)

    Wang, W.-B.; Zu, C.; He, L.; Zhang, W.-G.; Duan, L.-M.

    2015-07-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science.

  13. Memory-built-in quantum cloning in a hybrid solid-state spin register

    PubMed Central

    Wang, W.-B.; Zu, C.; He, L.; Zhang, W.-G.; Duan, L.-M.

    2015-01-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science. PMID:26178617

  14. Coherence and manipulation of spin states in semiconductor nanostructures

    NASA Astrophysics Data System (ADS)

    Gupta, Jay Anil

    Ultrafast optical techniques are developed to study and control carrier spin dynamics in semiconductor quantum dots and wells. Systematic studies of spin relaxation were performed in CdSe quantum dots (QDs) ranging from 22--80A in diameter. A fundamental motivation for the experiments was to identify operative spin scattering pathways for carriers in semiconductors with the discrete bandstructure resulting from quantum confinement. Because carriers are physically isolated from one another by imbedding the QDs in an insulating matrix, these studies explore a novel system where homogeneous spin-spin interactions may be negligible. Disparate transverse and longitudinal spin relaxation was characterized by applying a magnetic field either perpendicular or parallel to the observation direction. Nanosecond-scale transverse spin lifetimes were observed that exhibit relatively little dependence on temperature up to 300K. Spin precession occurs at distinct frequencies that are attributed to electron and exciton spins. Transverse spin relaxation is shown to be limited by inhomogeneous dephasing through a proportionate reduction in spin lifetime with field. In contrast, longitudinal spin relaxation times increase with field, with a component that persists for >20mus at low temperatures <50K. Similar measurements in a related system of CdS1-xSex QDs suggest a possible connection between the mus-scale dynamics and interactions of carriers with nuclear spins. In an effort to identify and eliminate the limitations on transverse spin lifetimes imposed by sample inhomogeneity, an all-optical method was developed with the potential for producing pulse sequences familiar from conventional magnetic resonance that can reverse certain types of dephasing. An effective magnetic field was generated in a semiconductor quantum well by a 'tipping' pulse whose energy was tuned below the bandgap. Through the resultant optical Stark effect, magnetic field strengths of order 20T are achievable

  15. Conduction and Spin Transport via Edge States in Randomly Hydrogenated Graphene Nano-Ribbon

    NASA Astrophysics Data System (ADS)

    Inuzuka, Kohei; Honda, Syuta; Sano, Nobuyuki

    An edge state of σ-band of minority spin channel is developed in the band gap in a non-hydrogenated graphene nano-ribbon (GNR). The spin-resolved conductance via this edge state in the metal/graphene/metal junctions is analyzed by using the tight-binding approach. This conductance exponentially decreases with increasing hydrogenation at the edge of GNR. When the hydrogenation percentages at the edge are lesser than 70%, the spin-polarized conductance is produced. The spin-polarizability approaches -1 as the difference of hydrogenation percentages at two edges increase.

  16. Charge-density-wave stripe state in fractional quantum spin Hall effects

    NASA Astrophysics Data System (ADS)

    Li, Wei; Chen, Yan

    2016-02-01

    By means of finite-size exact diagonalization, we theoretically study the effect of an inter-spin interaction in a fractional quantum spin Hall system, and demonstrate that the charge-density-wave stripe state can be realized in a fractional quantum spin Hall system by tuning the strength of an inter-spin interaction, which clarifies the nature of the puzzling mysterious phase emerging in previous studies. The experimental realization of such exotic quantum state as well as its evolution in optical lattices are also discussed. These results may provide insights into the future studies of fractional topological insulators.

  17. Coherent state transfer between an electron and nuclear spin in (15)N@C(60).

    PubMed

    Brown, Richard M; Tyryshkin, Alexei M; Porfyrakis, Kyriakos; Gauger, Erik M; Lovett, Brendon W; Ardavan, Arzhang; Lyon, S A; Briggs, G Andrew D; Morton, John J L

    2011-03-18

    Electron spin qubits in molecular systems offer high reproducibility and the ability to self-assemble into larger architectures. However, interactions between neighboring qubits are "always on," and although the electron spin coherence times can be several hundred microseconds, these are still much shorter than typical times for nuclear spins. Here we implement an electron-nuclear hybrid scheme which uses coherent transfer between electron and nuclear spin degrees of freedom in order to both effectively turn on or off interqubit coupling mediated by dipolar interactions and benefit from the long nuclear spin decoherence times (T(2n)). We transfer qubit states between the electron and (15)N nuclear spin in (15)N@C(60) with a two-way process fidelity of 88%, using a series of tuned microwave and radio frequency pulses and measure a nuclear spin coherence lifetime of over 100 ms.

  18. Benchmarking spin-state chemistry in starless core models

    NASA Astrophysics Data System (ADS)

    Sipilä, O.; Caselli, P.; Harju, J.

    2015-06-01

    Aims: We aim to present simulated chemical abundance profiles for a variety of important species, giving special attention to spin-state chemistry, in order to provide reference results to which present and future models can be compared. Methods: We employ gas-phase and gas-grain models to investigate chemical abundances in physical conditions that correspond to starless cores. To this end, we have developed new chemical reaction sets for both gas-phase and grain-surface chemistry, including the deuterated forms of species with up to six atoms and the spin-state chemistry of light ions and of the species involved in the ammonia and water formation networks. The physical model is kept simple to facilitate straightforward benchmarking of other models against the results of this paper. Results: We find that the ortho/para ratios of ammonia and water are similar in both gas-phase and gas-grain models, particularly at late times, implying that the ratios are determined by gas-phase processes. Furthermore, the ratios do not exhibit any strong dependence on core density. We derive late-time ortho/para ratios of ~0.5 for ammonia and ~1.6 for water. We find that including or excluding deuterium in the calculations has little effect on the abundances of non-deuterated species and on the ortho/para ratios of ammonia and water, especially in gas-phase models where deuteration is naturally hindered by the presence of abundant heavy elements. Although we study a rather narrow temperature range (10-20 K), we find strong temperature dependence in, e.g., deuteration and nitrogen chemistry. For example, the depletion timescale of ammonia is significantly reduced when the temperature is increased from 10 to 20 K; this is because the increase in temperature translates into increased accretion rates, while the very high binding energy of ammonia prevents it from being desorbed at 20 K. Appendices are available in electronic form at http://www.aanda.org

  19. Tristability arising from singlet-triplet and quartet spin states for dimeric Co(II)salen.

    PubMed

    Min, Kil Sik; Arthur, Jordan; Shum, William W; Bharathy, Muktha; zur Loye, Hans-Conrad; Miller, Joel S

    2009-06-01

    The magnetic behavior of N,N'-ethylenebis(salicylideniminato)cobalt(II) (Co(II)Salen, 1) has been reinvestigated and reveals spin-crossover behavior above 295 K. It has a singlet ground state and a triplet excited state at 30 K (21 cm(-1); 60 cal/mol) above the ground state, and at a higher temperature spin crossover to the quartet, a second excited state occurs.

  20. Surface-induced spin state locking of the [Fe(H2B(pz)2)2(bipy)] spin crossover complex

    NASA Astrophysics Data System (ADS)

    Beniwal, S.; Zhang, X.; Mu, S.; Naim, A.; Rosa, P.; Chastanet, G.; Létard, J.-F.; Liu, J.; Sterbinsky, G. E.; Arena, D. A.; Dowben, P. A.; Enders, A.

    2016-05-01

    Temperature- and coverage-dependent studies of the Au(1 1 1)-supported spin crossover Fe(II) complex (SCO) of the type [Fe(H2B(pz)2)2(bipy)] with a suite of surface-sensitive spectroscopy and microscopy tools show that the substrate inhibits thermally induced transitions of the molecular spin state, so that both high-spin and low-spin states are preserved far beyond the spin transition temperature of free molecules. Scanning tunneling microscopy confirms that [Fe(H2B(pz)2)2(bipy)] grows as ordered, molecular bilayer islands at sub-monolayer coverage and as disordered film at higher coverage. The temperature dependence of the electronic structure suggest that the SCO films exhibit a mixture of spin states at room temperature, but upon cooling below the spin crossover transition the film spin state is best described as a mix of high-spin and low-spin state molecules of a ratio that is constant. This locking of the spin state is most likely the result of a substrate-induced conformational change of the interfacial molecules, but it is estimated that also the intra-atomic electron-electron Coulomb correlation energy, or Hubbard correlation energy U, could be an additional contributing factor.

  1. Vortex states and spin textures of rotating spin-orbit-coupled Bose-Einstein condensates in a toroidal trap

    NASA Astrophysics Data System (ADS)

    Wang, Huan; Wen, Linghua; Yang, Hui; Shi, Chunxiao; Li, Jinghong

    2017-08-01

    We consider the ground-state properties of Rashba spin-orbit-coupled pseudo-spin-1/2 Bose-Einstein condensates (BECs) in a rotating two-dimensional (2D) toroidal trap. In the absence of spin-orbit coupling (SOC), the increasing rotation frequency enhances the creation of giant vortices for the initially miscible BECs, while it can lead to the formation of semiring density patterns with irregular hidden vortex structures for the initially immiscible BECs. Without rotation, strong 2D isotropic SOC yields a heliciform-stripe phase for the initially immiscible BECs. Combined effects of rotation, SOC, and interatomic interactions on the vortex structures and typical spin textures of the ground state of the system are discussed systematically. In particular, for a fixed rotation frequency above the critical value, the increasing isotropic SOC favors a visible vortex necklace in each component which is accompanied by a hidden giant vortex plus a (several) hidden vortex necklace(s) in the central region. In the case of one-dimensional anisotropic SOC, large SOC strength results in the generation of hidden linear vortex string and the transition from initial component separation (component mixing) to component mixing (component separation). Furthermore, the peculiar spin textures including skyrmion lattice, skyrmion pair and skyrmion string are revealed in this system.

  2. Refined entanglement concentration for electron-spin entangled cluster states with quantum-dot spins in optical microcavities

    NASA Astrophysics Data System (ADS)

    Du, Fang-Fang; Long, Gui-Lu

    2017-01-01

    We present a refined entanglement concentration protocol (ECP) for an arbitrary unknown less-entangled four-electron-spin cluster state by exploring the optical selection rules derived from the quantum-dot spins in one-sided optical microcavities. In our ECP, the parties obtain not only the four-electron-spin systems in the partial entanglement with two unknown parameters, but also the less-entangled two-electron-spin systems in the first step. Utilizing the above preserved systems as the resource for the second step of our ECP, the parties can obtain a standard cluster state by keeping the robust odd-parity instances with two parity-check gates. Meanwhile, the systems in the rest three instances can be used as the resource in the next round of our ECP. The success probability of our ECP is largely increased by iteration of the ECP process. Moreover, all the coefficients of our ECP are unknown for the parties without assistance of extra single electron-spin, so our ECP maybe has good applications in quantum communication network in the future.

  3. Spin Polarization of the ν=1 Quantum Hall State Via Optical Spectroscopy

    NASA Astrophysics Data System (ADS)

    Goldberg, B. B.

    1996-03-01

    Recent theoretical work has shown that the response of a 2DES with small g-factor in the spin-polarized state (ν=1) to a change of one quantum of magnetic flux is not a single-particle spin-flip excitation, but rather a macroscopic spin object called a Skyrmion or charged spin-texture excitation (CSTE).(S. L. Sondhi, A. Karlhede, S. A. Kivelson, and E. H. Rezayi, Phys. Rev. B 47), 16419 (1993); H. A. Fertig, L. Brey, R. Cote, and A. H. MacDonald, Phys. Rev. B 50, 11018 (1994) Evidence of these excitations have been recently observed in NMR and in tilted-field transport measurements.(S. E. Barrett, G. Dabbagh, L. N. Pfeiffer, K. W. West, and Z. Tycko, Phys. Rev. Lett. 74), 5112 (1995); A. Schmeller, J. P. Eisenstein, L. N. Pfeiffer, K. W. West, LANL Cond-mat preprint 9506133. They consist of a radial spin density distribution that is reversed at the center but gradually heals to the spin background over a distance of many magnetic lengths. With each particle in a nearly spin-aligned neighborhood, the exchange contribution lowers the energy of the CSTE relative to a single flipped spin. We present an experimental observation of Skyrmions in GaAs through the dramatic reduction in the degree of spin-polarization when the Fermi energy moves off the mid-point of the spin-gap of the lowest Landau level, ν=1. The degree of electron spin polarization as a function of ν is measured through interband magneto-absorption spectroscopy which distinguish the occupancy of the two electron spin-states. The spectra show quenching of absorption to the lower energy, spin-up electron band directly correlated to an increase in the higher energy, spin-down absorption at ν=1. This indicates the spin-up state fills with electrons while the spin-down state empties, providing a large spin-polarization Sz which exhibits a pronounced, symmetric decay when ν deviates from 1. The data provide a measurement of the absolute electron spin and are evidence for the presence of Skyrmion

  4. Generic helical edge states due to Rashba spin-orbit coupling in a topological insulator

    NASA Astrophysics Data System (ADS)

    Ortiz, Laura; Molina, Rafael A.; Platero, Gloria; Lunde, Anders Mathias

    2016-05-01

    We study the helical edge states of a two-dimensional topological insulator without axial spin symmetry due to the Rashba spin-orbit interaction. Lack of axial spin symmetry can lead to so-called generic helical edge states, which have energy-dependent spin orientation. This opens the possibility of inelastic backscattering and thereby nonquantized transport. Here we find analytically the new dispersion relations and the energy dependent spin orientation of the generic helical edge states in the presence of Rashba spin-orbit coupling within the Bernevig-Hughes-Zhang model, for both a single isolated edge and for a finite width ribbon. In the single-edge case, we analytically quantify the energy dependence of the spin orientation, which turns out to be weak for a realistic HgTe quantum well. Nevertheless, finite size effects combined with Rashba spin-orbit coupling result in two avoided crossings in the energy dispersions, where the spin orientation variation of the edge states is very significantly increased for realistic parameters. Finally, our analytical results are found to compare well to a numerical tight-binding regularization of the model.

  5. All-Optical Formation of Coherent Dark States of Silicon-Vacancy Spins in Diamond

    NASA Astrophysics Data System (ADS)

    Pingault, Benjamin; Becker, Jonas N.; Schulte, Carsten H. H.; Arend, Carsten; Hepp, Christian; Godde, Tillmann; Tartakovskii, Alexander I.; Markham, Matthew; Becher, Christoph; Atatüre, Mete

    2014-12-01

    Spin impurities in diamond can be versatile tools for a wide range of solid-state-based quantum technologies, but finding spin impurities that offer sufficient quality in both photonic and spin properties remains a challenge for this pursuit. The silicon-vacancy center has recently attracted much interest because of its spin-accessible optical transitions and the quality of its optical spectrum. Complementing these properties, spin coherence is essential for the suitability of this center as a spin-photon quantum interface. Here, we report all-optical generation of coherent superpositions of spin states in the ground state of a negatively charged silicon-vacancy center using coherent population trapping. Our measurements reveal a characteristic spin coherence time, T2* , exceeding 45 nanoseconds at 4 K. We further investigate the role of phonon-mediated coupling between orbital states as a source of irreversible decoherence. Our results indicate the feasibility of all-optical coherent control of silicon-vacancy spins using ultrafast laser pulses.

  6. Ultrafast control of nuclear spins using only microwave pulses: Towards switchable solid-state quantum gates

    SciTech Connect

    Mitrikas, George; Sanakis, Yiannis; Papavassiliou, Georgios

    2010-02-15

    We demonstrate the control of the {alpha}-proton nuclear spin, I =1/2, coupled to the stable radical {center_dot}CH(COOH){sub 2}, S =1/2, in a {gamma}-irradiated malonic acid single crystal using only microwave pulses. We show that, depending on the state of the electron spin (m{sub S}={+-}1/2), the nuclear spin can be locked in a desired state or oscillate between m{sub I}=+1/2 and m{sub I}=-1/2 on the nanosecond time scale. This approach provides a fast way of controlling nuclear spin qubits and also enables the design of switchable spin-based quantum gates by addressing only the electron spin.

  7. Disordered ground states in a quantum frustrated spin chain with side chains

    NASA Astrophysics Data System (ADS)

    Takano, Ken'Ichi; Hida, Kazuo

    2008-04-01

    We study a frustrated mixed spin chain with side chains, where the spin species and the exchange interactions are spatially varied. A nonlinear σ model method is formulated for this model, and a phase diagram with two disordered spin-gap phases is obtained for typical cases. Among them, we examine the case with a main chain, which consists of an alternating array of spin-1 and spin- (1)/(2) sites, and side chains, each of which consists of a single spin- (1)/(2) site, in great detail. Based on numerical, perturbational, and variational approaches, we propose a singlet cluster solid picture for each phase, where the ground state is expressed as a tensor product of local singlet states.

  8. Low-temperature Spin-Ice State of Quantum Heisenberg Magnets on Pyrochlore Lattice

    NASA Astrophysics Data System (ADS)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    We establish that the isotropic spin-1/2 Heisenberg antiferromagnet on pyrochlore lattice enters a spin-ice state at low, but finite, temperature. Our conclusions are based on results of the bold diagrammatic Monte Carlo simulations that demonstrate good convergence of the skeleton series down to temperature T = J/6. The ``smoking gun'' identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for static spin-spin correlation function between the quantum Heisenberg and classical Heisenberg/Ising models at all accessible temperatures. In particular, at T/J = 1/6, the momentum dependence shows a characteristic bow-tie pattern with pinch points. By numerical analytical continuation method, we also obtain the dynamic structure factor at real frequencies, showing a diffusive spinon dynamics at pinch points and spin wave continuum along the nodal lines.?

  9. Numerical methods for computing the ground state of spin-1 Bose-Einstein condensates in a uniform magnetic field.

    PubMed

    Lim, Fong Yin; Bao, Weizhu

    2008-12-01

    We propose efficient and accurate numerical methods for computing the ground-state solution of spin-1 Bose-Einstein condensates subjected to a uniform magnetic field. The key idea in designing the numerical method is based on the normalized gradient flow with the introduction of a third normalization condition, together with two physical constraints on the conservation of total mass and conservation of total magnetization. Different treatments of the Zeeman energy terms are found to yield different numerical accuracies and stabilities. Numerical comparison between different numerical schemes is made, and the best scheme is identified. The numerical scheme is then applied to compute the condensate ground state in a harmonic plus optical lattice potential, and the effect of the periodic potential, in particular to the relative population of each hyperfine component, is investigated through comparison to the condensate ground state in a pure harmonic trap.

  10. Spin-Orbit Coupling Controlled J =3 /2 Electronic Ground State in 5 d3 Oxides

    NASA Astrophysics Data System (ADS)

    Taylor, A. E.; Calder, S.; Morrow, R.; Feng, H. L.; Upton, M. H.; Lumsden, M. D.; Yamaura, K.; Woodward, P. M.; Christianson, A. D.

    2017-05-01

    Entanglement of spin and orbital degrees of freedom drives the formation of novel quantum and topological physical states. Here we report resonant inelastic x-ray scattering measurements of the transition metal oxides Ca3 LiOsO6 and Ba2 YOsO6 , which reveals a dramatic spitting of the t2 g manifold. We invoke an intermediate coupling approach that incorporates both spin-orbit coupling and electron-electron interactions on an even footing and reveal that the ground state of 5 d3-based compounds, which has remained elusive in previously applied models, is a novel spin-orbit entangled J =3 /2 electronic ground state. This work reveals the hidden diversity of spin-orbit controlled ground states in 5 d systems and introduces a new arena in the search for spin-orbit controlled phases of matter.

  11. Time-bin state transfer to electron spin coherence in solids

    SciTech Connect

    Kosaka, Hideo; Inagaki, Takahiro; Hitomi, Ryuta; Izawa, Fumishige; Mitsumori, Yasuyoshi; Edamatsu, Keiichi; Rikitake, Yoshiaki; Imamura, Hiroshi

    2014-12-04

    We demonstrate that a coherent superposition state of two temporally separated optical pulses, called a time-bin state, can be transferred to that of up/down electron spins in a semiconductor by synchronizing the time separation to the precession period of either electrons or holes. The time-bin transfer scheme does not require polarization mode degeneracy and can map the time-bin state to the electron spin state that is not accessible directly using only polarization. The scheme offers a new approach for quantum interfaces between photons and electron spins.

  12. Measuring hole spin states of single quantum dot in germanium hut wire

    NASA Astrophysics Data System (ADS)

    Li, Shu-Xiao; Li, Yan; Gao, Fei; Xu, Gang; Li, Hai-Ou; Cao, Gang; Xiao, Ming; Wang, Ting; Zhang, Jian-Jun; Guo, Guo-Ping

    2017-03-01

    As a group IV material with confined holes, the germanium hut wire is considered a promising candidate for achieving fast electrically controlled spin qubits. Here we fabricated a single quantum dot device on a germanium hut wire and a standard charge stability diagram with excited states was observed by DC transport measurements. By analyzing the Zeeman splitting behaviors of each state, we chose a window for distinguishing different hole parities and spin states, launching the first step towards a useful spin qubit. Effective g-factors around 4.3 for both even and odd hole number states were also extracted.

  13. Zero level of a purely magnetic two-dimensional nonrelativistic Pauli operator for SPIN-1/2 particles

    NASA Astrophysics Data System (ADS)

    Grinevich, P. G.; Mironov, A. E.; Novikov, S. P.

    2010-09-01

    We study the manifold of complex Bloch-Floquet eigenfunctions for the zero level of a two-dimensional nonrelativistic Pauli operator describing the propagation of a charged particle in a periodic magnetic field with zero flux through the elementary cell and a zero electric field. We study this manifold in full detail for a wide class of algebraic-geometric operators. In the nonzero flux case, the Pauli operator ground state was found by Aharonov and Casher for fields rapidly decreasing at infinity and by Dubrovin and Novikov for periodic fields. Algebraic-geometric operators were not previously known for fields with nonzero flux because the complex continuation of "magnetic" Bloch-Floquet eigenfunctions behaves wildly at infinity. We construct several nonsingular algebraic-geometric periodic fields (with zero flux through the elementary cell) corresponding to complex Riemann surfaces of genus zero. For higher genera, we construct periodic operators with interesting magnetic fields and with the Aharonov-Bohm phenomenon. Algebraic-geometric solutions of genus zero also generate soliton-like nonsingular magnetic fields whose flux through a disc of radius R is proportional to R (and diverges slowly as R → ∞). In this case, we find the most interesting ground states in the Hilbert space L 2 (ℝ 2 ).

  14. Imaging electrical spin generation and spin Hall dynamics in semiconductors

    NASA Astrophysics Data System (ADS)

    Stern, N. P.

    2009-03-01

    The capability to generate and manipulate spin polarization through the spin-orbit interaction drives interest in all-electrical techniques to exploit electron spins for semiconductor spintronics. The spin Hall effect refers to the generation of a pure spin current transverse to a charge current, resulting in a spontaneous spin accumulation near sample boundaries without the need for magnetic fields or materials. Recent experiments toward imaging this electrically generated spin polarization with both spatially and temporally resolved Kerr rotation microscopy in bulk zincblende semiconductors are discussed. Both current-induced in-plane spin polarization and out-of-plane spin accumulation from the spin Hall effect are observed in ZnSe up to room temperatureootnotetextN. P. Stern, S. Ghosh, G. Xiang, M. Zhu, N. Samarth, and D. D. Awschalom, Phys. Rev. Lett. 97, 126603 (2006). In GaAs devices, spatially resolved measurements of steady-state spin Hall accumulation and associated modeling clarify the important role of drift and diffusion in transporting spins generated at sample boundaries to the device interiorootnotetextN. P. Stern, D. W. Steuerman, S. Mack, A. C. Gossard, and D. D. Awschalom, Appl. Phys. Lett. 91, 062109 (2007). In these typical optical experiments, electrically-generated spin accumulation is measured using steady-state techniques that do not directly observe dynamics at timescales important for device operation. Here we discuss a time- and spatially-resolved measurement of the spin Hall effect using a pulsed current to drive spin accumulationootnotetextN. P. Stern, D. W. Steuerman, S. Mack, A. C. Gossard, and D. D. Awschalom, Nat. Physics 4, 843 (2008). The dynamical processes of spin accumulation and diffusion reveal spatially-dependent nanosecond timescales comparable to the electric-field dependent spin coherence time. A time-dependent diffusion analysis reconciles the observed spatial and temporal dynamics of spin accumulation from the spin

  15. Proximity enhanced quantum spin Hall state in graphene

    SciTech Connect

    Kou, Liangzhi; Hu, Feiming; Yan, Binghai; Wehling, Tim; Felser, Claudia; Frauenheim, Thomas; Chen, Changfeng

    2015-02-23

    Graphene is the first model system of two-dimensional topological insulator (TI), also known as quantum spin Hall (QSH) insulator. The QSH effect in graphene, however, has eluded direct experimental detection because of its extremely small energy gap due to the weak spin–orbit coupling. Here we predict by ab initio calculations a giant (three orders of magnitude) proximity induced enhancement of the TI energy gap in the graphene layer that is sandwiched between thin slabs of Sb2Te3 (or MoTe2). This gap (1.5 meV) is accessible by existing experimental techniques, and it can be further enhanced by tuning the interlayer distance via compression. We reveal by a tight-binding study that the QSH state in graphene is driven by the Kane–Mele interaction in competition with Kekulé deformation and symmetry breaking. As a result, the present work identifies a new family of graphene-based TIs with an observable and controllable bulk energy gap in the graphene layer, thus opening a new avenue for direct verification and exploration of the long-sought QSH effect in graphene.

  16. Proximity enhanced quantum spin Hall state in graphene

    DOE PAGES

    Kou, Liangzhi; Hu, Feiming; Yan, Binghai; ...

    2015-02-23

    Graphene is the first model system of two-dimensional topological insulator (TI), also known as quantum spin Hall (QSH) insulator. The QSH effect in graphene, however, has eluded direct experimental detection because of its extremely small energy gap due to the weak spin–orbit coupling. Here we predict by ab initio calculations a giant (three orders of magnitude) proximity induced enhancement of the TI energy gap in the graphene layer that is sandwiched between thin slabs of Sb2Te3 (or MoTe2). This gap (1.5 meV) is accessible by existing experimental techniques, and it can be further enhanced by tuning the interlayer distance viamore » compression. We reveal by a tight-binding study that the QSH state in graphene is driven by the Kane–Mele interaction in competition with Kekulé deformation and symmetry breaking. As a result, the present work identifies a new family of graphene-based TIs with an observable and controllable bulk energy gap in the graphene layer, thus opening a new avenue for direct verification and exploration of the long-sought QSH effect in graphene.« less

  17. Single-spin entanglement

    NASA Astrophysics Data System (ADS)

    Furman, G. B.; Meerovich, V. M.; Sokolovsky, V. L.

    2017-09-01

    We show that the operators and the quadrupole and Zeeman Hamiltonians for a spin 3/2 can be represented in terms for a system of two coupling fictitious spins 1/2 using the Kronecker product of Pauli matrices. Particularly, the quadrupole Hamiltonian which describes the interaction of the nuclear quadrupole moment with an electric field gradient is represented as the Hamiltonian of the Ising model in a transverse selective magnetic field. The Zeeman Hamiltonian, which describes interaction of the nuclear spin with the external magnetic field, can be considered as the Hamiltonian of the Heisenberg model in a selective magnetic field. The total Hamiltonian can be interpreted as the Hamiltonian of 3 D Heisenberg model in an inhomogeneous magnetic field applied along the x-axis. The representation of a single spin 3/2 as two-spin 1/2 system allows us to study entanglement in the spin system. One of the features of the fictitious spin system is that, in both the pure and the mixed states, the concurrence tends to 0.5 with increase of an applied magnetic field. The representation of a spin 3/2 as a system of two coupling fictitious spins 1/2 and possibility of formation of the entangled states in this system open a way to the application of a single spin 3/2 in quantum computation.

  18. High-spin states and a new band based on the isomeric state in 152Nd

    NASA Astrophysics Data System (ADS)

    Yeoh, E. Y.; Zhu, S. J.; Hamilton, J. H.; Ramayya, A. V.; Yang, Y. C.; Sun, Y.; Hwang, J. K.; Liu, S. H.; Wang, J. G.; Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.; Ding, H. B.; Li, K.; Gu, L.; Xu, Q.; Xiao, Z. G.; Ma, W. C.

    2010-08-01

    High-spin states of the neutron-rich 152Nd nucleus have been reinvestigated by measuring the prompt γ -rays in the spontaneous fission of 252Cf . The ground-state band and a side negative-parity band have been updated. A new band based on the 2243.7keV isomeric state has been identified. The half-life for the isomeric state has been measured to be 63(7)ns. The projected shell model is employed to study the band structure of this nucleus. The results show that the calculated levels of the bands are in good agreement with the experimental ones, and the isomeric state and the negative-parity band are based on the proton π5/2-[532] ⊗ π9/2+[404] and neutron ν3/2-[521] ⊗ ν5/2+[642] two-quasiparticles configurations, respectively.

  19. High spin polarization and the origin of unique ferromagnetic ground state in CuFeSb

    SciTech Connect

    Sirohi, Anshu; Saha, Preetha; Gayen, Sirshendu; Gaurav, Abhishek; Jyotsna, Shubhra; Sheet, Goutam; Singh, Chandan K.; Kabir, Mukul; Thakur, Gohil S.; Haque, Zeba; Gupta, L. C.; Ganguli, Ashok K.

    2016-06-13

    CuFeSb is isostructural to the ferro-pnictide and chalcogenide superconductors and it is one of the few materials in the family that are known to stabilize in a ferromagnetic ground state. Majority of the members of this family are either superconductors or antiferromagnets. Therefore, CuFeSb may be used as an ideal source of spin polarized current in spin-transport devices involving pnictide and the chalcogenide superconductors. However, for that the Fermi surface of CuFeSb needs to be sufficiently spin polarized. In this paper we report direct measurement of transport spin polarization in CuFeSb by spin-resolved Andreev reflection spectroscopy. From a number of measurements using multiple superconducting tips we found that the intrinsic transport spin polarization in CuFeSb is high (∼47%). In order to understand the unique ground state of CuFeSb and the origin of large spin polarization at the Fermi level, we have evaluated the spin-polarized band structure of CuFeSb through first principles calculations. Apart from supporting the observed 47% transport spin polarization, such calculations also indicate that the Sb-Fe-Sb angles and the height of Sb from the Fe plane are strikingly different for CuFeSb than the equivalent parameters in other members of the same family thereby explaining the origin of the unique ground state of CuFeSb.

  20. Revisiting spin-lattice relaxation time measurements for dilute spins in high-resolution solid-state NMR spectroscopy.

    PubMed

    Fu, Riqiang; Li, Jun; Cui, Jingyu; Peng, Xinhua

    2016-07-01

    Numerous nuclear magnetic resonance (NMR) measurements of spin-lattice relaxation times (T1S) for dilute spins such as (13)C have led to investigations of the motional dynamics of individual functional groups in solid materials. In this work, we revisit the Solomon equations and analyze how the heteronuclear cross relaxation between the dilute S (e.g. (13)C) and abundant I (e.g. (1)H) spins affects the measured T1S values in solid-state NMR in the absence of (1)H saturation during the recovery time. It is found theoretically that at the beginning of the S spin magnetization recovery, the existence of non-equilibrium I magnetization introduces the heteronuclear cross relaxation effect onto the recovery of the S spin magnetization and confirmed experimentally that such a heteronuclear cross relaxation effect results in the recovery overshoot phenomena for the dilute spins when T1S is on the same order of T1H, leading to inaccurate measurements of the T1S values. Even when T1S is ten times larger than T1H, the heteronuclear cross relaxation effect on the measured T1S values is still noticeable. Furthermore, this cross relaxation effect on recovery trajectory of the S spins can be manipulated and even suppressed by preparing the initial I and S magnetization, so as to obtain the accurate T1S values. A sample of natural abundance l-isoleucine powder has been used to demonstrate the T1S measurements and their corresponding measured T1C values under various experimental conditions.

  1. Generation of spin-dependent coherent states in a quantum wire

    NASA Astrophysics Data System (ADS)

    Pawłowski, J.; Szumniak, P.; Bednarek, S.

    2016-10-01

    We propose an all-electrically controlled nanodevice—a gated semiconductor nanowire—capable of generating a coherent state of a single electron trapped in a harmonic oscillator or superposition of such coherent states—the Schrödinger cat state. In the proposed scheme, the electron in the ground state of the harmonic potential is driven by resonantly oscillating Rashba spin-orbit coupling. This allows for the creation of the Schrödinger cat state with superposition amplitudes depending on the initial electron spin state. Such a method can be used for initialization of a single-spin qubit defined in a coherent state. The harmonic confinement potential along the InSb nanowire and the modulation of the Rashba spin-orbit coupling is obtained by proper gating. The results are supported by realistic three-dimensional time-dependent self-consistent Poisson-Schrödinger calculations.

  2. Bound states of fractionalized excitations in a modulated Kitaev spin liquid

    NASA Astrophysics Data System (ADS)

    Théveniaut, Hugo; Vojta, Matthias

    2017-08-01

    Fractionalization is a hallmark of spin-liquid behavior; it typically leads to response functions consisting of continua instead of sharp modes. However, microscopic processes can enable the formation of short-distance bound states of fractionalized excitations, despite asymptotic deconfinement. Here we study such bound-state formation for the Z2 spin liquid realized in Kitaev's honeycomb compass model, supplemented by a kekulé distortion of the lattice. Bound states between flux pairs and Majorana fermions form in the Majorana band gaps. We calculate the dynamic spin susceptibility and show that bound states lead to sharp modes in the magnetic response of the spin liquid, with the momentum dependence of the corresponding spectral weight encoding the internal symmetry of the bound state. As a byproduct, we also show that isolated fluxes may produce Majorana bound states at exactly zero energy. Generalizations and implications of the results are discussed.

  3. Delocalized Spin States in 2D Atomic Layers Realizing Enhanced Electrocatalytic Oxygen Evolution.

    PubMed

    Chen, Shichuan; Kang, Zhixiong; Hu, Xin; Zhang, Xiaodong; Wang, Hui; Xie, Junfeng; Zheng, XuSheng; Yan, Wensheng; Pan, Bicai; Xie, Yi

    2017-08-01

    The electrocatalytic activity of transition-metal-based compounds is strongly related to the spin states of metal atoms. However, the ways for regulation of spin states of catalysts are still limited, and the underlying relationship between the spin states and catalytic activities remains unclear. Herein, for the first time, by taking Ni(II) -based compounds without high or low spin states for example, it is shown that their spin states can be delocalized after introducing structural distortion to the atomic layers. The delocalized spin states for Ni atoms can provide not only high electrical conductivity but also low adsorption energy between the active sites and reaction intermediates for the system. As expected, the ultrathin nanosheets of nickel-chalcogenides with structural distortions show dramatically enhanced activity in electrocatalytic oxygen evolution compared to their corresponding bulk samples. This work establishes new way for the design of advanced electrocatalysts in transition-metal-based compounds via regulation of spin states. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  4. Spin Polarization and Attosecond Time Delay in Photoemission from Spin Degenerate States of Solids

    NASA Astrophysics Data System (ADS)

    Fanciulli, Mauro; Volfová, Henrieta; Muff, Stefan; Braun, Jürgen; Ebert, Hubert; Minár, Jan; Heinzmann, Ulrich; Dil, J. Hugo

    2017-02-01

    After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecond-resolved photoemission experiments. According to the Eisenbud-Wigner-Smith model, the time delay is due to a phase shift of different transitions that occur in the process. Such a phase shift is also at the origin of the angular dependent spin polarization of the photoelectron beam, observable in spin degenerate systems without angular momentum transfer by the incident photon. We propose a semiquantitative model which permits us to relate spin and time scales in photoemission from condensed matter targets and to better understand spin- and angle-resolved photoemission spectroscopy (SARPES) experiments on spin degenerate systems. We also present the first experimental determination by SARPES of this time delay in a dispersive band, which is found to be greater than 26 as for electrons emitted from the sp-bulk band of the model system Cu(111).

  5. Spin Polarization and Attosecond Time Delay in Photoemission from Spin Degenerate States of Solids.

    PubMed

    Fanciulli, Mauro; Volfová, Henrieta; Muff, Stefan; Braun, Jürgen; Ebert, Hubert; Minár, Jan; Heinzmann, Ulrich; Dil, J Hugo

    2017-02-10

    After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecond-resolved photoemission experiments. According to the Eisenbud-Wigner-Smith model, the time delay is due to a phase shift of different transitions that occur in the process. Such a phase shift is also at the origin of the angular dependent spin polarization of the photoelectron beam, observable in spin degenerate systems without angular momentum transfer by the incident photon. We propose a semiquantitative model which permits us to relate spin and time scales in photoemission from condensed matter targets and to better understand spin- and angle-resolved photoemission spectroscopy (SARPES) experiments on spin degenerate systems. We also present the first experimental determination by SARPES of this time delay in a dispersive band, which is found to be greater than 26 as for electrons emitted from the sp-bulk band of the model system Cu(111).

  6. Spin depolarization effect induced by charge state conversion of nitrogen vacancy center in diamond

    NASA Astrophysics Data System (ADS)

    Chen, Xiang-Dong; Zhou, Lei-Ming; Zou, Chang-Ling; Li, Cong-Cong; Dong, Yang; Sun, Fang-Wen; Guo, Guang-Can

    2015-09-01

    The electron spin of the negatively charged the nitrogen vacancy center (NV- ) in diamond can be optically polarized through intersystem crossing, which enables the defect to be used for quantum computation and metrology. In this work, we studied the electron spin depolarization effect of the NV center induced by charge state conversion, which was proven to be a spin-independent process. The spin-state initialization fidelity was largely affected by the charge state conversion process. As a result, the optical polarization of the electron spin decreased about 14 %(31 % ) with a high-power continuous-wave (pulsed) green laser. Moreover, the undefined fluorescence anomalous saturation effect of the NV center was analyzed and explained in detail based on the spin depolarization. The results demonstrated that a weak laser should be used for initialization of the NV center. In addition, the power and polarization of a laser for NV spin detection should be carefully adjusted to obtain the highest fluorescence signal. Our work also provided information that can increase the understanding of the charge state conversion and spin polarization processes of the NV center for quantum information and sensing.

  7. Experimental violation of a spin-1 bell inequality using maximally entangled four-photon states.

    PubMed

    Howell, John C; Lamas-Linares, Antia; Bouwmeester, Dik

    2002-01-21

    We demonstrate the experimental violation of a spin-1 Bell inequality. The spin-1 inequality is based on the Clauser, Horne, Shimony, and Holt formalism. For entangled spin-1 particles, the maximum quantum-mechanical prediction is 2.55 as opposed to a maximum of 2, predicted using local hidden variables. We obtained an experimental value of 2.27+/-0.02 using the four-photon state generated by pulsed, type-II, stimulated parametric down-conversion. This is a violation of the spin-1 Bell inequality by more than 13 standard deviations.

  8. Nuclear-spin-induced localization of edge states in two-dimensional topological insulators

    NASA Astrophysics Data System (ADS)

    Hsu, Chen-Hsuan; Stano, Peter; Klinovaja, Jelena; Loss, Daniel

    2017-08-01

    We investigate the influence of nuclear spins on the resistance of helical edge states of two-dimensional topological insulators (2DTIs). Via the hyperfine interaction, nuclear spins allow electron backscattering, otherwise forbidden by time-reversal symmetry. We identify two backscattering mechanisms, depending on whether the nuclear spins are ordered or not. Their temperature dependence is distinct but both give resistance, which increases with the edge length, decreasing temperature, and increasing strength of the electron-electron interaction. Overall, we find that the nuclear spins will typically shut down the conductance of the 2DTI edges at zero temperature.

  9. Magnetoresistance in the Spin-Orbit Kondo State of Elemental Bismuth

    PubMed Central

    Craco, Luis; Leoni, Stefano

    2015-01-01

    Materials with strong spin-orbit coupling, which competes with other particle-particle interactions and external perturbations, offer a promising route to explore novel phases of quantum matter. Using LDA + DMFT we reveal the complex interplay between local, multi-orbital Coulomb and spin-orbit interaction in elemental bismuth. Our theory quantifies the role played by collective dynamical fluctuations in the spin-orbit Kondo state. The correlated electronic structure we derive is promising in the sense that it leads to results that might explain why moderate magnetic fields can generate Dirac valleys and directional-selective magnetoresistance responses within spin-orbit Kondo metals. PMID:26358556

  10. A quaternionic map for the steady states of the Heisenberg spin-chain

    NASA Astrophysics Data System (ADS)

    Mehta, Mitaxi P.; Dutta, Souvik; Tiwari, Shubhanshu

    2014-01-01

    We show that the steady states of the classical Heisenberg XXX spin-chain in an external magnetic field can be found by iterations of a quaternionic map. A restricted model, e.g., the xy spin-chain is known to have spatially chaotic steady states and the phase space occupied by these chaotic states is known to go through discrete changes as the field strength is varied. The same phenomenon is studied for the xxx spin-chain. It is seen that in this model the phase space volume varies smoothly with the external field.

  11. Communication: Dissolution DNP reveals a long-lived deuterium spin state imbalance in methyl groups

    NASA Astrophysics Data System (ADS)

    Jhajharia, Aditya; Weber, Emmanuelle M. M.; Kempf, James G.; Abergel, Daniel; Bodenhausen, Geoffrey; Kurzbach, Dennis

    2017-01-01

    We report the generation and observation of long-lived spin states in deuterated methyl groups by dissolution DNP. These states are based on population imbalances between manifolds of spin states corresponding to irreducible representations of the C3v point group and feature strongly dampened quadrupolar relaxation. Their lifetime depends on the activation energies of methyl group rotation. With dissolution DNP, we can reduce the deuterium relaxation rate by a factor up to 20, thereby extending the experimentally available time window. The intrinsic limitation of NMR spectroscopy of quadrupolar spins by short relaxation times can thus be alleviated.

  12. Bound states in the continuum in spin-orbit-coupled atomic systems

    NASA Astrophysics Data System (ADS)

    Kartashov, Yaroslav V.; Konotop, Vladimir V.; Torner, Lluis

    2017-09-01

    We show that the interplay between spin-orbit coupling and Zeeman splitting in atomic systems can lead to the existence of bound states in the continuum (BICs) supported by trapping potentials. Such states have energies falling well within the continuum spectrum, but nevertheless they are localized and fully radiationless. We report the existence of BICs, in some cases in exact analytical form, in systems with tunable spin-orbit coupling and show that the phenomenon is physically robust. We also found that BIC states may be excited in spin-orbit-coupled Bose-Einstein condensates, where under suitable conditions they may be metastable with remarkably long lifetimes.

  13. Dimer-Monomer Ground State for Extended Spin-1/2 Diamond Chain

    NASA Astrophysics Data System (ADS)

    Takano, Ken'ichi

    2017-09-01

    We present a condition in which the dimer-monomer state is exactly the ground state of an extended diamond chain with spin magnitude 1/2. The Hamiltonian of the extended diamond chain includes next-nearest-neighbor exchange interactions and distortions, where the spin magnitude of the spin pair on a singlet dimer is not generally conserved. The method of deriving the condition is based on representing the Hamiltonian in a complete square form. The dimer-monomer ground state is found even if the Hamiltonian has no space-reflection symmetries.

  14. Quantum spin liquid ground states of the Heisenberg-Kitaev model on the triangular lattice

    NASA Astrophysics Data System (ADS)

    Kos, Pavel; Punk, Matthias

    2017-01-01

    We study quantum disordered ground states of the two-dimensional Heisenberg-Kitaev model on the triangular lattice using a Schwinger boson approach. Our aim is to identify and characterize potential gapped quantum spin liquid phases that are stabilized by anisotropic Kitaev interactions. For antiferromagnetic Heisenberg and Kitaev couplings and sufficiently small spin S , we find three different symmetric Z2 spin liquid phases, separated by two continuous quantum phase transitions. Interestingly, the gap of elementary excitations remains finite throughout the transitions. The first spin liquid phase corresponds to the well-known zero-flux state in the Heisenberg limit, which is stable with respect to small Kitaev couplings and develops 120∘ order in the semiclassical limit at large S . In the opposite Kitaev limit, we find a different spin liquid ground state, which is a quantum disordered version of a magnetically ordered state with antiferromagnetic chains, in accordance with results in the classical limit. Finally, at intermediate couplings, we find a spin liquid state with unusual spin correlations. Upon spinon condensation, this state develops Bragg peaks at incommensurate momenta in close analogy to the magnetically ordered Z2 vortex crystal phase, which has been analyzed in recent theoretical works.

  15. The spin state of iron in minerals of Earth's lower mantle

    SciTech Connect

    Sturhahn, Wolfgang; Jackson, Jennifer M.; Lin, Jung -Fu

    2005-06-23

    Here, the spin state of Fe(II) and Fe(III) at temperatures and pressures typical for the Earth's lower mantle is discussed. We predict an extended high-spin to low-spin crossover region along the geotherm for Fe-dilute systems depending on crystal-field splitting, pairing energy, and cooperative interactions. In particular, spin transitions in ferromagnesium silicate perovskite and ferropericlase, the dominant lower mantle components, should occur in a wide temperature-pressure range. We also derive a gradual volume change associated with such transitions in the lower mantle. The gradual density changes and the wide spin crossover regions seem incompatible with lower mantle stratification resulting from a spin transition.

  16. The spin state of iron in minerals of Earth's lower mantle

    DOE PAGES

    Sturhahn, Wolfgang; Jackson, Jennifer M.; Lin, Jung -Fu

    2005-06-23

    Here, the spin state of Fe(II) and Fe(III) at temperatures and pressures typical for the Earth's lower mantle is discussed. We predict an extended high-spin to low-spin crossover region along the geotherm for Fe-dilute systems depending on crystal-field splitting, pairing energy, and cooperative interactions. In particular, spin transitions in ferromagnesium silicate perovskite and ferropericlase, the dominant lower mantle components, should occur in a wide temperature-pressure range. We also derive a gradual volume change associated with such transitions in the lower mantle. The gradual density changes and the wide spin crossover regions seem incompatible with lower mantle stratification resulting from amore » spin transition.« less

  17. Nuclear Spin Relaxation in Glass States of 3He-A in Stretched Aerogel

    NASA Astrophysics Data System (ADS)

    Dmitriev, V. V.; Krasnikhin, D. A.; Mulders, N.; Senin, A. A.; Yudin, A. N.

    2011-02-01

    We present results of pulse NMR investigations of superfluid A-like phase of 3He in stretched aerogel. In this case we have anisotropic orbital glass (OG) with two possible types of ordering in spin space—ordered spin nematic (OG-SN) or disordered spin glass (OG-SG) states. It was found that longitudinal relaxation of magnetization is non-exponential in both states and depends on temperature and on inhomogeneity of external steady magnetic field. At the same conditions the relaxation in OG-SG state is more rapid than in OG-SN state. For transverse orientation of the magnetic field relative to anisotropy axis the duration of free induction decay signal was longer than in normal phase. It may be explained by formation of coherently precessing spin state.

  18. Persistent coherence and spin polarization of topological surface states on topological insulators

    NASA Astrophysics Data System (ADS)

    Pan, Z.-H.; Vescovo, E.; Fedorov, A. V.; Gu, G. D.; Valla, T.

    2013-07-01

    Gapless surface states on topological insulators are protected from elastic scattering on nonmagnetic impurities, which makes them promising candidates for low-power electronic applications. However, for widespread applications, these states should remain coherent and significantly spin polarized at ambient temperatures. Here, we studied the coherence and spin structure of the topological states on the surface of a model topological insulator, Bi2Se3, at elevated temperatures in spin- and angle-resolved photoemission spectroscopy. We found an extremely weak broadening and essentially no decay of spin polarization of the topological surface state up to room temperature. Our results demonstrate that the topological states on surfaces of topological insulators could serve as a basis for room-temperature electronic devices.

  19. Direct measurement of nonlocal entanglement of two-qubit spin quantum states.

    PubMed

    Cheng, Liu-Yong; Yang, Guo-Hui; Guo, Qi; Wang, Hong-Fu; Zhang, Shou

    2016-01-18

    We propose efficient schemes of direct concurrence measurement for two-qubit spin and photon-polarization entangled states via the interaction between single-photon pulses and nitrogen-vacancy (NV) centers in diamond embedded in optical microcavities. For different entangled-state types, diversified quantum devices and operations are designed accordingly. The initial unknown entangled states are possessed by two spatially separated participants, and nonlocal spin (polarization) entanglement can be measured with the aid of detection probabilities of photon (NV center) states. This non-demolition entanglement measurement manner makes initial entangled particle-pair avoid complete annihilation but evolve into corresponding maximally entangled states. Moreover, joint inter-qubit operation or global qubit readout is not required for the presented schemes and the final analyses inform favorable performance under the current parameters conditions in laboratory. The unique advantages of spin qubits assure our schemes wide potential applications in spin-based solid quantum information and computation.

  20. Direct measurement of nonlocal entanglement of two-qubit spin quantum states

    NASA Astrophysics Data System (ADS)

    Cheng, Liu-Yong; Yang, Guo-Hui; Guo, Qi; Wang, Hong-Fu; Zhang, Shou

    2016-01-01

    We propose efficient schemes of direct concurrence measurement for two-qubit spin and photon-polarization entangled states via the interaction between single-photon pulses and nitrogen-vacancy (NV) centers in diamond embedded in optical microcavities. For different entangled-state types, diversified quantum devices and operations are designed accordingly. The initial unknown entangled states are possessed by two spatially separated participants, and nonlocal spin (polarization) entanglement can be measured with the aid of detection probabilities of photon (NV center) states. This non-demolition entanglement measurement manner makes initial entangled particle-pair avoid complete annihilation but evolve into corresponding maximally entangled states. Moreover, joint inter-qubit operation or global qubit readout is not required for the presented schemes and the final analyses inform favorable performance under the current parameters conditions in laboratory. The unique advantages of spin qubits assure our schemes wide potential applications in spin-based solid quantum information and computation.

  1. Quantum metrology with entangled spin-coherent states of two modes

    NASA Astrophysics Data System (ADS)

    Berrada, K.; Khalek, S. Abdel; Ooi, C. H. Raymond

    2012-09-01

    Recently, Gerry [Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.79.022111 79, 022111 (2009)] studied the violation of the Bell-Clauser-Horne-Shimony-Holt inequality for two-spin systems, prepared in an entanglement of spin-coherent states, the so-called entangled spin-coherent states (ESCSs), and found maximal violations for a large class of states. In this paper, using the Holstein-Primakoff realization (HPR) of angular momentum algebra, we present an improved phase estimation scheme employing ESCSs and demonstrate that increasing the spin number gives the smallest variance in the phase parameter in comparison to NOON states under perfect and lossy conditions. The phase sensitivity of this interferometric scheme with parity detection on one of the output states is discussed.

  2. Double Charge Ordering States and Spin Ordering State Observed in a RFe2O4 System

    PubMed Central

    Sun, Fei; Wang, Rui; Aku-Leh, C.; Yang, H. X.; He, Rui; Zhao, Jimin

    2014-01-01

    Charge, spin, and lattice degrees of orderings are of great interest in the layered quantum material RFe2O4 (R = Y, Er, Yb, Tm, and Lu) system. Recently many unique properties have been found using various experimental methods. However so far the nature of the two-dimensional (2D) charge ordering (CO) state is not clear and no observation of its fine structure in energy has been reported. Here we report unambiguous observation of double 2D CO states at relatively high temperature in a polycrystalline Er0.1Yb0.9Fe2O4 using Raman scattering. The energy gaps between the 3D and the double 2D states are 170 meV (41.2 THz) and 193 meV (46.6 THz), respectively. We also observed a spin ordering (SO) state at below 210 K with characteristic energy of 45 meV (10.7 THz). Our investigation experimentally identified new fine structures of quantum orders in the system, which also extends the capability of optical methods in investigating other layered quantum materials. PMID:25234133

  3. Nanoscale self-hosting of molecular spin-states in the intermediate phase of a spin-crossover material.

    PubMed

    Bréfuel, Nicolas; Collet, Eric; Watanabe, Hiroshi; Kojima, Masaaki; Matsumoto, Naohide; Toupet, Loic; Tanaka, Koichiro; Tuchagues, Jean-Pierre

    2010-12-17

    A new spin-crossover (SC) complex [Fe(II)H(2)L(2-Me)][AsF(6)](2) has been synthesized, in which H(2)L(2-Me) denotes the chirogenic hexadentate N(6) Schiff-base ligand bis{[(2-methylimidazol-4-yl)methylidene]-3-aminopropyl}ethylenediamine. This complex has revealed a rich variety of phases during its two-step thermal crossover, as well as photoinduced spin-state switching. A high-symmetry high-spin (HS, S=2) phase, a low-symmetry low-spin (LS, S=0) phase, an intermediate phase characterized by an unprecedented lozenge pattern of 12 predominantly HS molecular crystallographic sites confining 18 predominantly LS molecular crystallographic sites, and a photoinduced low-symmetry HS phase have been accurately evidenced by temperature-dependent magnetic susceptibility, Mössbauer spectroscopy, and crystallographic studies. This variety of phases illustrates the multi-stability of this system, which results from coupling between the electronic states and structural instabilities.

  4. Critical competition between two distinct orbital-spin ordered states in perovskite vanadates

    NASA Astrophysics Data System (ADS)

    Fujioka, J.; Yasue, T.; Miyasaka, S.; Yamasaki, Y.; Arima, T.; Sagayama, H.; Inami, T.; Ishii, K.; Tokura, Y.

    2010-10-01

    We have investigated the spin/orbital phase diagram in the perovskite orthovanadate RVO3 ( R=Eu , Y, Dy, and Ho) by measurements of magnetization, dielectric constant, specific heat, Raman scattering spectra, and x-ray diffraction, focusing on the interplay between the V3d spin and the 4f moment of the R ion. The thermally induced phase transition between the C-type spin/G-type orbital ordered state and the G-type spin/C-type orbital ordered state is observed for Eu1-xYxVO3 (x=0-0.52) without 4f moment. By comparing this phase diagram with the spin/orbital ordering in TbVO3 , it is evident that the critical competition between the C-type spin/G-type orbital ordered phase and the G-type spin/C-type orbital ordered one depends not only on the GdFeO3 -type lattice distortion but also on the presence of the 4f moment of the R ion. The magnetic field induced phase transition of the spin/orbital ordering is achieved concomitantly with polarizing R4f moments for DyVO3 and HoVO3 . For DyVO3 , the G-type spin/C-type orbital ordered phase is switched to the C-type spin/G-type orbital ordered one by applying a moderate magnetic field around 3 T. By contrast, the G-type spin/C-type orbital ordering is rather favored under the magnetic field in HoVO3 . The results cannot be uniquely explained in terms of the exchange interaction between the V3d spin and the R -ion 4f moment. The coupling of the R4f moment polarization with the lattice distortion tied with the orbital ordering of the V3d sublattice may also be relevant to this field induced phase transition.

  5. Intricacies of the Co3 + spin state in Sr2Co0.5Ir0.5O4 : An x-ray absorption and magnetic circular dichroism study

    NASA Astrophysics Data System (ADS)

    Agrestini, S.; Kuo, C.-Y.; Mikhailova, D.; Chen, K.; Ohresser, P.; Pi, T. W.; Guo, H.; Komarek, A. C.; Tanaka, A.; Hu, Z.; Tjeng, L. H.

    2017-06-01

    We report on a combined soft x-ray absorption and magnetic circular dichroism (XMCD) study at the Co-L3 ,2 edge on the hybrid 3 d /5 d solid state oxide Sr2Co0.5Ir0.5O4 with K2NiF4 structure. Our data indicate unambiguously a pure high spin state (S =2 ) for the Co3 + (3 d6 ) ions with a significant unquenched orbital moment Lz/2 Sz=0.25 despite the sizable elongation of the CoO6 octahedra. Using quantitative model calculations based on parameters consistent with our spectra, we have investigated the stability of this high spin state with respect to the competing low spin and intermediate spin states.

  6. Quantum model of a solid-state spin qubit: Ni cluster on a silicon surface by the generalized spin Hamiltonian and X-ray absorption spectroscopy investigations

    NASA Astrophysics Data System (ADS)

    Farberovich, Oleg V.; Mazalova, Victoria L.; Soldatov, Alexander V.

    2015-11-01

    We present here the quantum model of a Ni solid-state electron spin qubit on a silicon surface with the use of a density-functional scheme for the calculation of the exchange integrals in the non-collinear spin configurations in the generalized spin Hamiltonian (GSH) with the anisotropic exchange coupling parameters linking the nickel ions with a silicon substrate. In this model the interaction of a spin qubit with substrate is considered in GSH at the calculation of exchange integrals Jij of the nanosystem Ni7-Si in the one-electron approach taking into account chemical bonds of all Si-atoms of a substrate (environment) with atoms of the Ni7-cluster. The energy pattern was found from the effective GSH Hamiltonian acting in the restricted spin space of the Ni ions by the application of the irreducible tensor operators (ITO) technique. In this paper we offer the model of the quantum solid-state N-spin qubit based on the studying of the spin structure and the spin-dynamics simulations of the 3d-metal Ni clusters on the silicon surface. The solution of the problem of the entanglement between spin states in the N-spin systems is becoming more interesting when considering clusters or molecules with a spectral gap in their density of states. For quantifying the distribution of the entanglement between the individual spin eigenvalues (modes) in the spin structure of the N-spin system we use the density of entanglement (DOE). In this study we have developed and used the advanced high-precision numerical techniques to accurately assess the details of the decoherence process governing the dynamics of the N-spin qubits interacting with a silicon surface. We have studied the Rabi oscillations to evaluate the N-spin qubits system as a function of the time and the magnetic field. We have observed the stabilized Rabi oscillations and have stabilized the quantum dynamical qubit state and Rabi driving after a fixed time (0.327 μs). The comparison of the energy pattern with the

  7. Quantum filter of spin polarized states: Metal–dielectric–ferromagnetic/semiconductor device

    SciTech Connect

    Makarov, Vladimir I.; Khmelinskii, Igor

    2014-02-01

    Highlights: • Development of a new spintronics device. • Development of quantum spin polarized filters. • Development of theory of quantum spin polarized filter. - Abstract: Recently we proposed a model for the Quantum Spin-Polarized State Filter (QSPSF). The magnetic moments are transported selectively in this model, detached from the electric charge carriers. Thus, transfer of a spin-polarized state between two conductors was predicted in a system of two levels coupled by exchange interaction. The strength of the exchange interaction between the two conductive layers depends on the thickness of the dielectric layer separating them. External magnetic fields modulate spin-polarized state transfer, due to Zeeman level shift. Therefore, a linearly growing magnetic field generates a series of current peaks in a nearby coil. Thus, our spin-state filter should contain as least three nanolayers: (1) conductive or ferromagnetic; (2) dielectric; and (3) conductive or semiconductive. The spectrum of spin-polarized states generated by the filter device consists of a series of resonance peaks. In a simple case the number of lines equals S, the total spin angular momentum of discrete states in one of the coupled nanolayers. Presently we report spin-polarized state transport in metal–dielectric–ferromagnetic (MDF) and metal–dielectric–semiconductor (MDS) three-layer sandwich devices. The exchange-resonance spectra in such devices are quite specific, differing also from spectra observed earlier in other three-layer devices. The theoretical model is used to interpret the available experimental results. A detailed ab initio analysis of the magnetic-field dependence of the output magnetic moment averaged over the surface of the device was carried out. The model predicts the resonance structure of the signal, although at its present accuracy it cannot predict the positions of the spectral peaks.

  8. Spin to Charge Interconversion Phenomena in the Interface and Surface States

    NASA Astrophysics Data System (ADS)

    Ando, Yuichiro; Shiraishi, Masashi

    2017-01-01

    In 1985, Johnson and Silsbee realized the creation of a spin current in nonmagnetic metals, which inspired a vast number of studies related to the spin current until now. Creation of the spin current has been realized in metals, semiconductors, and insulators to date and has provided a fruitful research field. Spin-dependent conductance and spin torque paved a new way for spintronic application, and highly efficient interconversion between spin information and an industrially used one, such as charge current, light, magnetic moment and heat current, became a central topic. In the early stage, the main field of such interconversion was bulk materials; the focus then gradually shifted to surface and interface states. The properties of surface and interface states became pronounced in nanoscale spintronics devices, and a variety of functions have been realized at the interface between two materials, enabling limitless possibilities for spin functions. This review provides an overview of the recent progress of the spin-charge interconversion in the surface and interface states. We also introduce several spurious effects that should be paid careful attention for quantitative investigations.

  9. Improved spin squeezing of an atomic ensemble through internal state control

    NASA Astrophysics Data System (ADS)

    Hemmer, Daniel; Montano, Enrique; Deutsch, Ivan; Jessen, Poul

    2016-05-01

    Squeezing of collective atomic spins is typically generated by quantum backaction from a QND measurement of the relevant spin component. In this scenario the degree of squeezing is determined by the measurement resolution relative to the quantum projection noise (QPN) of a spin coherent state (SCS). Greater squeezing can be achieved through optimization of the 3D geometry of probe and atom cloud, or by placing the atoms in an optical cavity. We explore here a complementary strategy that relies on quantum control of the large internal spin available in alkali atoms such as Cs. Using a combination of rf and uw magnetic fields, we coherently map the internal spins in our ensemble from the SCS (| f = 4, m = 4>) to a ``cat'' state which is an equal superposition of | f = 4, m = 4>and | f = 4, m = -4>. This increases QPN by a factor of 2 f = 8 relative to the SCS, and therefore the amount of backaction and spin-spin entanglement produced by our QND measurement. In a final step, squeezing generated in the cat state basis can be mapped back to the SCS basis, where it corresponds to increased squeezing of the physical spin. Our experiments suggest that up to 8dB of metrologically useful squeezing can be generated in this way, compared to ~ 3 dB in an otherwise identical experiment starting from a SCS.

  10. Mechanism of dilute-spin-exchange in solid-state NMR

    SciTech Connect

    Lu, George J.; Opella, Stanley J.

    2014-03-28

    In the stationary, aligned samples used in oriented sample (OS) solid-state NMR, {sup 1}H-{sup 1}H homonuclear dipolar couplings are not attenuated as they are in magic angle spinning solid-state NMR; consequently, they are available for participation in dipolar coupling-based spin-exchange processes. Here we describe analytically the pathways of {sup 15}N-{sup 15}N spin-exchange mediated by {sup 1}H-{sup 1}H homonuclear dipolar couplings. The mixed-order proton-relay mechanism can be differentiated from the third spin assisted recoupling mechanism by setting the {sup 1}H to an off-resonance frequency so that it is at the “magic angle” during the spin-exchange interval in the experiment, since the “magic angle” irradiation nearly quenches the former but only slightly attenuates the latter. Experimental spectra from a single crystal of N-acetyl leucine confirm that this proton-relay mechanism plays the dominant role in {sup 15}N-{sup 15}N dilute-spin-exchange in OS solid-state NMR in crystalline samples. Remarkably, the “forbidden” spin-exchange condition under “magic angle” irradiation results in {sup 15}N-{sup 15}N cross-peaks intensities that are comparable to those observed with on-resonance irradiation in applications to proteins. The mechanism of the proton relay in dilute-spin-exchange is crucial for the design of polarization transfer experiments.

  11. Spin-state blockade in Te6+-substituted electron-doped LaCoO3

    NASA Astrophysics Data System (ADS)

    Tomiyasu, Keisuke; Koyama, Shun-Ichi; Watahiki, Masanori; Sato, Mika; Nishihara, Kazuki; Onodera, Mitsugi; Iwasa, Kazuaki; Nojima, Tsutomu; Yamasaki, Yuuichi; Nakao, Hironori; Murakami, Youichi

    2015-03-01

    Perovskite-type LaCoO3 (Co3+: d6) is a rare inorganic material with sensitive and characteristic responses among low, intermediate, and high spin states. For example, in insulating nonmagnetic low-spin states below about 20 K, light hole doping (Ni substitution) induces much larger magnetization than expected; over net 10μB/hole (5μB/Ni) for 1μB/hole (1μB/Ni), in which the nearly isolated dopants locally change the surrounding Co low-spin states to magnetic ones and form spin molecules with larger total spin. Further, the former is isotropic, whereas the latter exhibits characteristic anisotropy probably because of Jahn-Teller distortion. In contrast, for electron doping, relatively insensitive spin-state responses were reported, as in LaCo(Ti4+) O3, but are not clarified, and are somewhat controversial. Here, we present macroscopic measurement data of another electron-doped system LaCo(Te6+) O3 and discuss the spin-state responses. This study was financially supported by Grants-in-Aid for Young Scientists (B) (No. 22740209 and 26800174) from the MEXT of Japan.

  12. Noise-induced collective quantum state preservation in spin qubit arrays

    NASA Astrophysics Data System (ADS)

    Barnes, Edwin; Deng, Dong-Ling; Throckmorton, Robert E.; Wu, Yang-Le; Das Sarma, S.

    2016-02-01

    The hyperfine interaction with nuclear spins (or, Overhauser noise) has long been viewed as a leading source of decoherence in individual quantum dot spin qubits. Here we show that in a coupled multiqubit system consisting of as few as four spins, interactions with nuclear spins can have the opposite effect where they instead preserve the collective quantum state of the system. This noise-induced state preservation can be realized in a linear spin qubit array using current technological capabilities. Our proposal requires no control over the Overhauser fields in the array; only experimental control over the average interqubit coupling between nearest neighbors is needed, and this is readily achieved by tuning gate voltages. Our results illustrate how the role of the environment can transform from harmful to helpful in the progression from single-qubit to multiqubit quantum systems.

  13. Noise-induced collective quantum state preservation in spin qubit arrays

    NASA Astrophysics Data System (ADS)

    Barnes, Edwin; Deng, Dong-Ling; Throckmorton, Robert; Wu, Yang-Le

    The hyperfine interaction with nuclear spins (or, Overhauser noise) has long been viewed as a leading source of decoherence in individual quantum dot spin qubits. We show that in a coupled multi-qubit system consisting of as few as four spins, interactions with nuclear spins can have the opposite effect where they instead preserve the collective quantum state of the system. This noise-induced state preservation can be realized in a linear spin qubit array using current technological capabilities. Our proposal requires no control over the Overhauser fields in the array; only experimental control over the average interqubit coupling between nearest neighbors is needed, and this is readily achieved by tuning gate voltages. Our results illustrate how the role of the environment can transform from harmful to helpful in the progression from single-qubit to multi-qubit quantum systems. Work supported by LPS-MPO-CMTC and IARPA-MQCO.

  14. Ground-state cooling of a carbon nanomechanical resonator by spin-polarized current.

    PubMed

    Stadler, P; Belzig, W; Rastelli, G

    2014-07-25

    We study the nonequilibrium steady state of a mechanical resonator in the quantum regime realized by a suspended carbon nanotube quantum dot in contact with two ferromagnets. Because of the spin-orbit interaction and/or an external magnetic field gradient, the spin on the dot couples directly to the flexural eigenmodes. Accordingly, the nanomechanical motion induces inelastic spin flips of the tunneling electrons. A spin-polarized current at finite bias voltage causes either heating or active cooling of the mechanical modes. We show that maximal cooling is achieved at resonant transport when the energy splitting between two dot levels of opposite spin equals the vibrational frequency. Even for weak electron-resonator coupling and moderate polarizations we can achieve ground-state cooling with a temperature of the leads, for instance, of T = 10 ω.

  15. Muon Spin Relaxation Evidence for the U(1) Quantum Spin-Liquid Ground State in the Triangular Antiferromagnet YbMgGaO_{4}.

    PubMed

    Li, Yuesheng; Adroja, Devashibhai; Biswas, Pabitra K; Baker, Peter J; Zhang, Qian; Liu, Juanjuan; Tsirlin, Alexander A; Gegenwart, Philipp; Zhang, Qingming

    2016-08-26

    Muon spin relaxation (μSR) experiments on single crystals of the structurally perfect triangular antiferromagnet YbMgGaO_{4} indicate the absence of both static long-range magnetic order and spin freezing down to 0.048 K in a zero field. Below 0.4 K, the μ^{+} spin relaxation rates, which are proportional to the dynamic correlation function of the Yb^{3+} spins, exhibit temperature-independent plateaus. All these μSR results unequivocally support the formation of a gapless U(1) quantum spin liquid ground state in the triangular antiferromagnet YbMgGaO_{4}.

  16. Spin-Projected Matrix Product States: Versatile Tool for Strongly Correlated Systems.

    PubMed

    Li, Zhendong; Chan, Garnet Kin-Lic

    2017-06-13

    We present a new wave function ansatz that combines the strengths of spin projection with the language of matrix product states (MPS) and matrix product operators (MPO) as used in the density matrix renormalization group (DMRG). Specifically, spin-projected matrix product states (SP-MPS) are constructed as [Formula: see text], where [Formula: see text] is the spin projector for total spin S and |ΨMPS((N,M))⟩ is an MPS wave function with a given particle number N and spin projection M. This new ansatz possesses several attractive features: (1) It provides a much simpler route to achieve spin adaptation (i.e., to create eigenfunctions of Ŝ(2)) compared to explicitly incorporating the non-Abelian SU(2) symmetry into the MPS. In particular, since the underlying state |ΨMPS((N,M))⟩ in the SP-MPS uses only Abelian symmetries, one does not need the singlet embedding scheme for nonsinglet states, as normally employed in spin-adapted DMRG, to achieve a single consistent variationally optimized state. (2) Due to the use of |ΨMPS((N,M))⟩ as its underlying state, the SP-MPS can be closely connected to broken-symmetry mean-field states. This allows one to straightforwardly generate the large number of broken-symmetry guesses needed to explore complex electronic landscapes in magnetic systems. Further, this connection can be exploited in the future development of quantum embedding theories for open-shell systems. (3) The sum of MPOs representation for the Hamiltonian and spin projector [Formula: see text] naturally leads to an embarrassingly parallel algorithm for computing expectation values and optimizing SP-MPS. (4) Optimizing SP-MPS belongs to the variation-after-projection (VAP) class of spin-projected theories. Unlike usual spin-projected theories based on determinants, the SP-MPS ansatz can be made essentially exact simply by increasing the bond dimensions in |ΨMPS((N,M))⟩. Computing excited states is also simple by imposing orthogonality constraints, which

  17. Universal scheme for finite-probability perfect transfer of arbitrary multispin states through spin chains

    SciTech Connect

    Man, Zhong-Xiao; An, Nguyen Ba; Xia, Yun-Jie; Kim, Jaewan

    2014-12-15

    In combination with the theories of open system and quantum recovering measurement, we propose a quantum state transfer scheme using spin chains by performing two sequential operations: a projective measurement on the spins of ‘environment’ followed by suitably designed quantum recovering measurements on the spins of interest. The scheme allows perfect transfer of arbitrary multispin states through multiple parallel spin chains with finite probability. Our scheme is universal in the sense that it is state-independent and applicable to any model possessing spin–spin interactions. We also present possible methods to implement the required measurements taking into account the current experimental technologies. As applications, we consider two typical models for which the probabilities of perfect state transfer are found to be reasonably high at optimally chosen moments during the time evolution. - Highlights: • Scheme that can achieve perfect quantum state transfer is devised. • The scheme is state-independent and applicable to any spin-interaction models. • The scheme allows perfect transfer of arbitrary multispin states. • Applications to two typical models are considered in detail.

  18. New high spin states and isomers in the {sup 208}Pb and {sup 207}Pb nuclei

    SciTech Connect

    Broda, R.; Wrzesinski, J.; Pawlat, T.

    1996-12-31

    The two most prominent examples of the heavy doubly closed shell (DCS) nuclei, {sup 208}Pb and {sup 132}Sn, are not accessible by conventional heavy-ion fusion processes populating high-spin states. This experimental difficulty obscured for a long time the investigation of yrast high-spin states in both DCS and neighboring nuclei and consequently restricted the study of the shell model in its most attractive regions. Recent technical development of multidetector gamma arrays opened new ways to exploit more complex nuclear processes which populate the nuclei of interest with suitable yields for gamma spectroscopy and involve population of moderately high spin states. This new possibility extended the range of accessible spin values and is a promising way to reach new yrast states. Some of these states are expected to be of high configurational purity and can be a source of important shell model parameters which possibly can be used later to check the validity of the spherical shell model description at yet higher spin and higher excitation energy. The nuclei in the closest vicinity of {sup 132}Sn are produced in spontaneous fission and states with spin values up to I=14 can be reached in fission gamma spectroscopy studies with the presently achieved sensitivity of gamma arrays. New results on yrast states in the {sup 134}Te and {sup 135}I nuclei populated in fission of the {sup 248}Cm presented at this conference illustrate such application of the resolving power offered by modern gamma techniques.

  19. Entanglement of two-electron spin states in a double quantum dot

    NASA Astrophysics Data System (ADS)

    Bagrov, V. G.; Gitman, D. M.; Levin, A. D.; Meireles, M. S.

    Recently, an implementation of a universal set of one- and two-quantum-bit gates for quantum computation using spin states of coupled single-electron quantum dots was proposed. It was demonstrated that it is possible to execute a coherent control of a quantum system based on two-electron spin states in a double quantum dot, allowing state preparation, coherent manipulation, and projective readout. This possibility is based on rapid electrical control of the spin exchange interaction. These results motivated us to develop a formal theoretical study of the corresponding model of two coupled spins placed in a magnetic field and subjected to a time-dependent mutual Heisenberg interaction. Using possible exact solutions of the corresponding quantum problem, we study entangling of different separable initial states in this model. It is demonstrated that the entanglement due to a time-dependent Heisenberg interaction is dominating in comparison with the entanglement due to the action of an external magnetic field.

  20. Spin texture of time-reversal symmetry invariant surface states on W(110)

    PubMed Central

    Kutnyakhov, D.; Chernov, S.; Medjanik, K.; Wallauer, R.; Tusche, C.; Ellguth, M.; Nepijko, S. A.; Krivenkov, M.; Braun, J.; Borek, S.; Minár, J.; Ebert, H.; Elmers, H. J.; Schönhense, G.

    2016-01-01

    We find in the case of W(110) previously overlooked anomalous surface states having their spin locked at right angle to their momentum using spin-resolved momentum microscopy. In addition to the well known Dirac-like surface state with Rashba spin texture near the -point, we observe a tilted Dirac cone with circularly shaped cross section and a Dirac crossing at 0.28 ×   within the projected bulk band gap of tungsten. This state has eye-catching similarities to the spin-locked surface state of a topological insulator. The experiments are fortified by a one-step photoemission calculation in its density-matrix formulation. PMID:27406652

  1. High-spin states in the five-valence-particle nucleus {sup 213}Po

    SciTech Connect

    Astier, Alain; Porquet, Marie-Genevieve

    2011-03-15

    Excited states in {sup 213}Po have been populated using the {sup 18}O+ {sup 208}Pb reaction at 85 MeV beam energy and studied with the Euroball IV {gamma} multidetector array. The level scheme has been built up to {approx}2.0 MeV excitation energy and spin I{approx}25/2({h_bar}/2{pi}) from the triple {gamma} coincidence data. Spin and parity values of several yrast states have been assigned from the {gamma} angular properties. The configurations of the yrast states are discussed using results of empirical shell-model calculations and by analogy with the neighboring nuclei. The spin and parity values of several low-spin states of {sup 213}Po previously identified from the {beta} decay of {sup 213}Bi are revised.

  2. Electronic Structure of a Low-spin Heme/Cu Peroxide Complex: Spin-State and Spin-Topology Contributions to Reactivity

    PubMed Central

    Kieber-Emmons, Matthew T.; Li, Yuqi; Halime, Zakaria; Karlin, Kenneth D.; Solomon, Edward I.

    2011-01-01

    This study details the electronic structure of the heme-peroxo-copper adduct {[(F8)Fe(DCHIm)]-O2-[Cu(AN)]}+ (LSAN) in which O22− bridges the metals in a μ-1,2 or “end-on” configuration. LSAN is generated by addition of coordinating base to the parent complex {[(F8)Fe]-O2-[Cu(AN)]}+ (HSAN) in which the O22− bridges the metals in an μ-η2:η2 or “side-on” mode. In addition to the structural change of the O22− bridging geometry, coordination of the base changes the spin state of the heme fragment (from S = 5/2 in HSAN to S = 1/2 in LSAN) that results in an anti-ferromagnetically coupled diamagnetic ground state in LSAN. The strong ligand field of the porphyrin modulates the high-spin to low-spin effect on Fe-peroxo bonding relative to non-heme complexes, which is important in the O—O bond cleavage process. Based on DFT calculations, the ground state of LSAN is dependent on the Fe—O—O—Cu dihedral angle, wherein acute angles (< ~150°) yield an anti-ferromagnetically coupled electronic structure, while more obtuse angles yield a ferromagnetic ground state. LSAN is diamagnetic, and thus has an antiferromagnetically coupled ground state with a calculated Fe—O—O—Cu dihedral angle of 137°. The nature of the bonding in LSAN, and the frontier molecular orbitals which lead to this magneto-structural correlation, provide insight into possible spin topology contributions to O—O bond cleavage by cytochrome c oxidase. PMID:22007669

  3. Feasible Perturbations of Control Systems with Pure State Constraints and Applications to Second-Order Optimality Conditions

    SciTech Connect

    Hoehener, Daniel

    2013-10-15

    We propose second-order necessary optimality conditions for optimal control problems with very general state and control constraints which hold true under weak regularity assumptions on the data. In particular the pure state constraints are general closed sets, the optimal control is supposed to be merely measurable and the dynamics may be discontinuous in the time variable as well. These results are obtained by an approach based on local perturbations of the reference process by second-order tangent directions. This method allows direct and quite simple proofs.

  4. Mechanical control of spin states in single molecules

    NASA Astrophysics Data System (ADS)

    Parks, J. J.; Champagne, A. R.; Costi, T. A.; Pasupathy, A. N.; Shum, W. W.; Neuscamman, E.; Chan, G. K.-L.; Abruña, H. D.; Ralph, D. C.

    2010-03-01

    We study individual Co(tpy-SH)2 complexes by connecting them within mechanically controllable break-junction devices that allow us to controllably stretch the molecule while measuring its electrical conductance. At low temperature, this molecule produces the Kondo effect, observed as a peak in the conductance at zero bias. We find that as a function of stretching the Kondo peak splits in two, in distinct contrast to behavior observed in spin-1/2 molecules. The temperature dependence of the Kondo signal for the unstretched molecule is in agreement with the scaling prediction for an underscreened S = 1 Kondo effect. The splitting of the Kondo resonance by mechanical stretching can be explained by a spin-orbit-induced lifting of the degeneracy of the S = 1 triplet upon distortion from octahedral symmetry of the Co ion. We observe evidence of the resultant spin anisotropy in the magnetic-field dependence of the Kondo peaks.

  5. A Manifold of Pure Gibbs States of the Ising Model on the Lobachevsky Plane

    NASA Astrophysics Data System (ADS)

    Gandolfo, Daniel; Ruiz, Jean; Shlosman, Senya

    2015-02-01

    In this paper we construct many `new' Gibbs states of the Ising model on the Lobachevsky plane, the millefeuilles. Unlike the usual states on the integer lattices, our foliated states have infinitely many interfaces. The interfaces are rigid and fill the Lobachevsky plane with positive density. We also construct analogous states on the Cayley trees.

  6. Generation of Quality Pulses for Control of Qubit/Quantum Memory Spin States: Experimental and Simulation

    DTIC Science & Technology

    2016-09-01

    nuclear spin states of qubits/quantum memory applicable to semiconductor, superconductor, ionic, and superconductor-ionic hybrid technologies. As the...multiplexer. The output of the multiplexer is amplified and then passed into a directional coupler. One output is passed through a schottky diode and...electronic control circuitry for control of electron/nuclear spin states of qubits/quantum memory applicable to semiconductor, superconductor, ionic

  7. Tunable symmetry breaking and helical edge transport in a graphene quantum spin Hall state.

    PubMed

    Young, A F; Sanchez-Yamagishi, J D; Hunt, B; Choi, S H; Watanabe, K; Taniguchi, T; Ashoori, R C; Jarillo-Herrero, P

    2014-01-23

    Low-dimensional electronic systems have traditionally been obtained by electrostatically confining electrons, either in heterostructures or in intrinsically nanoscale materials such as single molecules, nanowires and graphene. Recently, a new method has emerged with the recognition that symmetry-protected topological (SPT) phases, which occur in systems with an energy gap to quasiparticle excitations (such as insulators or superconductors), can host robust surface states that remain gapless as long as the relevant global symmetry remains unbroken. The nature of the charge carriers in SPT surface states is intimately tied to the symmetry of the bulk, resulting in one- and two-dimensional electronic systems with novel properties. For example, time reversal symmetry endows the massless charge carriers on the surface of a three-dimensional topological insulator with helicity, fixing the orientation of their spin relative to their momentum. Weakly breaking this symmetry generates a gap on the surface, resulting in charge carriers with finite effective mass and exotic spin textures. Analogous manipulations have yet to be demonstrated in two-dimensional topological insulators, where the primary example of a SPT phase is the quantum spin Hall state. Here we demonstrate experimentally that charge-neutral monolayer graphene has a quantum spin Hall state when it is subjected to a very large magnetic field angled with respect to the graphene plane. In contrast to time-reversal-symmetric systems, this state is protected by a symmetry of planar spin rotations that emerges as electron spins in a half-filled Landau level are polarized by the large magnetic field. The properties of the resulting helical edge states can be modulated by balancing the applied field against an intrinsic antiferromagnetic instability, which tends to spontaneously break the spin-rotation symmetry. In the resulting canted antiferromagnetic state, we observe transport signatures of gapped edge states

  8. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    DOE PAGES

    Marino, Andrea; Buron-Le Cointe, M.; Lorenc, M.; ...

    2015-01-28

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. Lastly, by combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW

  9. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    SciTech Connect

    Marino, Andrea; Buron-Le Cointe, M.; Lorenc, M.; Toupet, L.; Henning, Robert W.; DiChiara, A. D.; Moffat, Keith; Brefuel, N.; Collet, E.

    2015-01-28

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. Lastly, by combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW

  10. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves.

    PubMed

    Marino, A; Buron-Le Cointe, M; Lorenc, M; Toupet, L; Henning, R; DiChiara, A D; Moffat, K; Bréfuel, N; Collet, E

    2015-01-01

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. By combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW.

  11. Confinement of spin-orbit induced Dirac states in quantum point contacts

    NASA Astrophysics Data System (ADS)

    Li, Tommy

    2015-08-01

    The quantum transmission problem for a particle moving in a quantum point contact in the presence of a Rashba spin-orbit interaction and applied magnetic field is solved semiclassically. A strong Rashba interaction and parallel magnetic field form emergent Dirac states at the center of the constriction, leading to the appearance of resonances which carry spin current and become bound at high magnetic fields. These states can be controlled in situ by modulation of external electric and magnetic fields, and can be used to turn the channel into a spin pump which operates at zero bias. It is shown that this effect is currently experimentally accessible in p -type quantum point contacts.

  12. NMR Search for the Spin Nematic State in a LaFeAsO Single Crystal

    NASA Astrophysics Data System (ADS)

    Fu, M.; Torchetti, D. A.; Imai, T.; Ning, F. L.; Yan, J.-Q.; Sefat, A. S.

    2012-12-01

    We report a As75 single crystal NMR investigation of LaFeAsO, the parent phase of a pnictide high Tc superconductor. We demonstrate that spin dynamics develop a strong twofold anisotropy within each orthorhombic domain below the tetragonal-orthorhombic structural phase transition at TTO≈156K. This intermediate state with a dynamical breaking of the rotational symmetry freezes progressively into a spin density wave below TSDW≈142K. Our findings are consistent with the presence of a spin nematic state below TTO with an incipient magnetic order.

  13. Optical detection and ionization of donors in specific electronic and nuclear spin States.

    PubMed

    Yang, A; Steger, M; Karaiskaj, D; Thewalt, M L W; Cardona, M; Itoh, K M; Riemann, H; Abrosimov, N V; Churbanov, M F; Gusev, A V; Bulanov, A D; Kaliteevskii, A K; Godisov, O N; Becker, P; Pohl, H-J; Ager, J W; Haller, E E

    2006-12-01

    We resolve the remarkably sharp bound exciton transitions of highly enriched 28Si using a single-frequency laser and photoluminescence excitation spectroscopy, as well as photocurrent spectroscopy. Well-resolved doublets in the spectrum of the 31P donor reflect the hyperfine coupling of the electronic and nuclear donor spins. The optical detection of the nuclear spin state, and selective pumping and ionization of donors in specific electronic and nuclear spin states, suggests a number of new possibilities which could be useful for the realization of silicon-based quantum computers.

  14. Entangled electron and nuclear spin states in 15N@C60: Density matrix tomography

    NASA Astrophysics Data System (ADS)

    Scherer, Werner; Mehring, Michael

    2008-02-01

    Procedures of the preparation and detection of entangled electron-nuclear spin states in N15@C60 by combining electron spin resonance and electron nuclear double resonance pulse techniques are presented. A quantitative evaluation of the complete density matrix is obtained by a special density matrix tomography. All four Bell states of a two qubit subsystem were analyzed and experimental decoherence times are presented. In addition, we estimate a quantum critical temperature of Tq=7.76K for this system at an electron spin resonance frequency of 95GHz.

  15. Crossover from an incommensurate singlet spiral state with a vanishingly small spin gap to a valence-bond solid state in dimerized frustrated ferromagnetic spin chains

    NASA Astrophysics Data System (ADS)

    Agrapidis, Cliò Efthimia; Drechsler, Stefan-Ludwig; van den Brink, Jeroen; Nishimoto, Satoshi

    2017-06-01

    Motivated by the magnetic properties of the spin-chain compounds LiCuSbO4≡LiSbCuO4 and Rb2Cu2Mo3O12 , we study the ground state of the Heisenberg chain with dimerized nearest-neighbor ferromagnetic (FM) (J1,J1'<0 ) and next-nearest-neighbor antiferromagnetic (J2>0 ) couplings. Using the density-matrix renormalization group technique and spin-wave theory, we find a first-order transition between a fully polarized FM and an incommensurate spiral state at 2 α =β /(1 +β ) , where α is the frustration ratio J2/|J1| and β the degree of dimerization J1'/J1 . In the singlet spiral state the spin-gap is vanishingly small in the vicinity of the FM transition, corresponding to a situation of LiCuSbO4. For larger α , corresponding to Rb2Cu2Mo3O12 , and smaller β there is a crossover from this frustration induced incommensurate state to an Affleck-Lieb-Kennedy-Tasaki-type valence-bond solid state with substantial spin gaps.

  16. Spin glass behavior in frustrated quantum spin system CuAl 2 O 4 with a possible orbital liquid state

    DOE PAGES

    Nirmala, R.; Jang, Kwang-Hyun; Sim, Hasung; ...

    2017-02-15

    CuAl2O4 is a normal spinel oxide having quantum spin, S = 1/2 for Cu2+. It is a rather unique feature that the Cu2+ ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it exhibits all the thermodynamic evidence of a quantum spin glass. For example, the polycrystalline CuAl2O4 shows a cusp centered at ~2 K in the low-field dc magnetization data and a clear frequency dependence in the ac magnetic susceptibility while it displays logarithmic relaxation behavior in a time dependence of the magnetization. At the same time, theremore » is a peak at ~2.3 K in the heat capacity, which shifts towards a higher temperature with magnetic fields. Conversely, there is no evidence of new superlattice peaks in the high-resolution neutron powder diffraction data when cooled from 40 to 0.4 K. This implies that there is no long-ranged magnetic order down to 0.4 K, thus confirming a spin glass-like ground state for CuAl2O4. Interestingly, there is no sign of structural distortion either although Cu2+ is a Jahn–Teller active ion. Therefore, we claim that an orbital liquid state is the most likely ground state in CuAl2O4. Of further interest, it also exhibits a large frustration parameter, f = |θ CW/T m| ~ 67, one of the largest values reported for spinel oxides. These observations suggest that CuAl2O4 should be a rare example of a frustrated quantum spin glass with a good candidate for an orbital liquid state.« less

  17. Spin glass behavior in frustrated quantum spin system CuAl2O4 with a possible orbital liquid state

    NASA Astrophysics Data System (ADS)

    Nirmala, R.; Jang, Kwang-Hyun; Sim, Hasung; Cho, Hwanbeom; Lee, Junghwan; Yang, Nam-Geun; Lee, Seongsu; Ibberson, R. M.; Kakurai, K.; Matsuda, M.; Cheong, S.-W.; Gapontsev, V. V.; Streltsov, S. V.; Park, Je-Geun

    2017-04-01

    CuAl2O4 is a normal spinel oxide having quantum spin, S  =  1/2 for Cu2+. It is a rather unique feature that the Cu2+ ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it exhibits all the thermodynamic evidence of a quantum spin glass. For example, the polycrystalline CuAl2O4 shows a cusp centered at ~2 K in the low-field dc magnetization data and a clear frequency dependence in the ac magnetic susceptibility while it displays logarithmic relaxation behavior in a time dependence of the magnetization. At the same time, there is a peak at ~2.3 K in the heat capacity, which shifts towards a higher temperature with magnetic fields. On the other hand, there is no evidence of new superlattice peaks in the high-resolution neutron powder diffraction data when cooled from 40 to 0.4 K. This implies that there is no long-ranged magnetic order down to 0.4 K, thus confirming a spin glass-like ground state for CuAl2O4. Interestingly, there is no sign of structural distortion either although Cu2+ is a Jahn–Teller active ion. Thus, we claim that an orbital liquid state is the most likely ground state in CuAl2O4. Of further interest, it also exhibits a large frustration parameter, f  =  |θ CW/T m| ~ 67, one of the largest values reported for spinel oxides. Our observations suggest that CuAl2O4 should be a rare example of a frustrated quantum spin glass with a good candidate for an orbital liquid state.

  18. Spin glass behavior in frustrated quantum spin system CuAl2O4 with a possible orbital liquid state.

    PubMed

    Nirmala, R; Jang, Kwang-Hyun; Sim, Hasung; Cho, Hwanbeom; Lee, Junghwan; Yang, Nam-Geun; Lee, Seongsu; Ibberson, R M; Kakurai, K; Matsuda, M; Cheong, S-W; Gapontsev, V V; Streltsov, S V; Park, Je-Geun

    2017-04-05

    CuAl2O4 is a normal spinel oxide having quantum spin, S  =  1/2 for Cu(2+). It is a rather unique feature that the Cu(2+) ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it exhibits all the thermodynamic evidence of a quantum spin glass. For example, the polycrystalline CuAl2O4 shows a cusp centered at ~2 K in the low-field dc magnetization data and a clear frequency dependence in the ac magnetic susceptibility while it displays logarithmic relaxation behavior in a time dependence of the magnetization. At the same time, there is a peak at ~2.3 K in the heat capacity, which shifts towards a higher temperature with magnetic fields. On the other hand, there is no evidence of new superlattice peaks in the high-resolution neutron powder diffraction data when cooled from 40 to 0.4 K. This implies that there is no long-ranged magnetic order down to 0.4 K, thus confirming a spin glass-like ground state for CuAl2O4. Interestingly, there is no sign of structural distortion either although Cu(2+) is a Jahn-Teller active ion. Thus, we claim that an orbital liquid state is the most likely ground state in CuAl2O4. Of further interest, it also exhibits a large frustration parameter, f  =  |θ CW/T m| ~ 67, one of the largest values reported for spinel oxides. Our observations suggest that CuAl2O4 should be a rare example of a frustrated quantum spin glass with a good candidate for an orbital liquid state.

  19. Cavity QED with magnetically coupled collective spin states.

    PubMed

    Amsüss, R; Koller, Ch; Nöbauer, T; Putz, S; Rotter, S; Sandner, K; Schneider, S; Schramböck, M; Steinhauser, G; Ritsch, H; Schmiedmayer, J; Majer, J

    2011-08-05

    We report strong coupling between an ensemble of nitrogen-vacancy center electron spins in diamond and a superconducting microwave coplanar waveguide resonator. The characteristic scaling of the collective coupling strength with the square root of the number of emitters is observed directly. Additionally, we measure hyperfine coupling to (13)C nuclear spins, which is a first step towards a nuclear ensemble quantum memory. Using the dispersive shift of the cavity resonance frequency, we measure the relaxation time of the NV center at millikelvin temperatures in a nondestructive way.

  20. Interface states in two-dimensional electron systems with spin-orbital interaction.

    PubMed

    Sukhanov, Aleksei A; Sablikov, Vladimir A

    2011-10-05

    Interface states at a boundary between regions with different spin-orbit interactions (SOIs) in two-dimensional (2D) electron systems are investigated within the one-band effective mass method with generalized boundary conditions for envelope functions. We have found that the interface states unexpectedly exist even if the effective interface potential equals zero. Depending on the system parameters, the energy of these states can lie in either or both forbidden and conduction bands of bulk states. The interface states have chiral spin texture similar to that of the edge states in 2D topological insulators. However, their energy spectrum is more sensitive to the interfacial potential, the largest effect being produced by the spin-dependent component of the interfacial potential. We have also studied the size quantization of the interface states in a strip of 2D electron gas with SOI and found an unusual (non-monotonic) dependence of the quantization energy on the strip width.