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Sample records for pwo scintillation crystals

  1. Characterization and Recovery of Lead Tungstate (PWO4) Crystals

    NASA Astrophysics Data System (ADS)

    McShane, Abigail; Griggs, Dannie

    2016-09-01

    The potential of Lead Tungstate (PWO) crystals in EM calorimeters like the Neutral Particle Spectrometer at 12 GeV JLab and future particle identification detectors of the Electron Ion Collider has been researched extensively. The small Moliere radius of PWO crystals make them ideal for use in a compact detector and their light yield outperforms that of other heavy crystals. Recent measurements have shown large variations in crystal properties. This is a major concern for the construction of particle identification detectors. Testing of the crystal uniformity and understanding the origin of the variation have thus become necessary. The characterization of PWO includes measurements of the crystal dimensions, optical transmittance, both longitudinal and transverse, the light yield and decay kinetics to identify slow luminescence components, as well as tests of radiation hardness. Optical clarity after radiation damage can in principle be restored by stimulated recovery with light. Optical bleaching with blue light is the default method, but curing at longer wavelength may be possible. The results of crystal characterization and effects of radiation on optical properties, as well as the effectiveness and practicality of the LED curing system will be discussed. This work was supported in part by NSF Grant PHY-1306227.

  2. Application of two-photon absorption in PWO scintillator for fast timing of interaction with ionizing radiation

    NASA Astrophysics Data System (ADS)

    Auffray, E.; Buganov, O.; Korjik, M.; Fedorov, A.; Nargelas, S.; Tamulaitis, G.; Tikhomirov, S.; Vaitkevičius, A.

    2015-12-01

    This work was aimed at searching for fast phenomena in scintillators in sub-10-ps range, a benchmark timing for the time response of radiation detectors in particle colliders. The pump-and-probe optical absorption technique with a tunable-wavelength parametric oscillator as the pump and a continuous-spectrum source as the probe beam was used to study lead tungstate PbWO4 (PWO) single crystals. It is shown that the rise time of the probe pulse absorption induced by the pump pulse is shorter than the pump pulse width of 200 fs. The approximately linear dependence of the probe absorption on the pump pulse energy density evidences that the induced absorption is caused by two-photon absorption involving one probe and one pump photon. We demonstrate that the intensity of the induced absorption at certain wavelengths is influenced by gamma irradiation, provided that an appropriate light polarization is selected. The application of the irradiation-sensitive nonlinearity for fast timing in radiation detectors is discussed.

  3. Scintillation of lead tungstate crystal studied with single-electron beam from KUFEL

    SciTech Connect

    Rizwan, Mohamad Uozumi, Yusuke; Matsuo, Kazuki; Ohgaki, Hideaki; Kii, Toshiteru; Zen, Heishun; Tsamalaidze, Zviadi; Evtoukhovitch, Petr; Valentin, Samoilov

    2015-04-29

    Lead tungstate (PWO) crystal has a very fast response, high atomic density and high radiation hardness. Therefore, they are suitable to be used for high-energy nuclear data measurements under high-background circumstances. Although a good electron-ion separation with a pulse shape analysis technique is essential, scintillation pulse shapes have not been observed with electron beams of a wide energy range. A single-electron beam technique has been developed at Kyoto University Free Electron Laser (KUFEL), and electron beams of 4-38 MeV are available. During the experiments, single electron beams bombarded a PWO crystal. By using oscilloscope we observed scintillation pulses of a PWO crystal coupled with a photomultiplier tube. Measured spectra were compared with the simulation code of EGS5 to analyze scattering effects. As the result, the pulse amplitudes show good linearity and the pulse shapes are almost constant in the observed energy range.

  4. Mixed crystal organic scintillators

    DOEpatents

    Zaitseva, Natalia P; Carman, M Leslie; Glenn, Andrew M; Hamel, Sebastien; Hatarik, Robert; Payne, Stephen A; Stoeffl, Wolfgang

    2014-09-16

    A mixed organic crystal according to one embodiment includes a single mixed crystal having two compounds with different bandgap energies, the organic crystal having a physical property of exhibiting a signal response signature for neutrons from a radioactive source, wherein the signal response signature does not include a significantly-delayed luminescence characteristic of neutrons interacting with the organic crystal relative to a luminescence characteristic of gamma rays interacting with the organic crystal. According to one embodiment, an organic crystal includes bibenzyl and stilbene or a stilbene derivative, the organic crystal having a physical property of exhibiting a signal response signature for neutrons from a radioactive source.

  5. Investigating the Anisotropic Scintillation Response in Organic Crystal Scintillator Detectors

    NASA Astrophysics Data System (ADS)

    Schuster, Patricia Frances

    This dissertation presents several studies that experimentally characterize the scintillation anisotropy in organic crystal scintillators. These include measurements of neutron, gamma-ray and cosmic muon interactions in anthracene, a historical benchmark among organic scintillator materials, to confirm and extend measurements previously available in the literature. The gamma-ray and muon measurements provide new experimental confirmation that no scintillation anisotropy is present in their interactions. Observations from these measurements have updated the hypothesis for the physical mechanism that is responsible for the scintillation anisotropy concluding that a relatively high dE/dx is required in order to produce a scintillation anisotropy. The directional dependence of the scintillation output in liquid and plastic materials was measured to experimentally confirm that no scintillation anisotropy correlated to detector orientation exists in amorphous materials. These observations confirm that the scintillation anisotropy is not due to an external effect on the measurement system, and that a fixed, repeating structure is required for a scintillation anisotropy. The directional dependence of the scintillation output in response to neutron interactions was measured in four stilbene crystals of various sizes and growth-methods. The scintillation anisotropy in these materials was approximately uniform, indicating that the crystal size, geometry, and growth method do not significantly impact the effect. Measurements of three additional pure crystals and two mixed crystals were made. These measurements showed that 1) the magnitude of the effect varies with energy and material, 2) the relationship between the light output and pulse shape anisotropy varies across materials, and 3) the effect in mixed materials is very complex. These measurements have informed the hypothesis of the mechanism that produces the directional dependence. By comparing the various relationships

  6. Photonic crystal scintillators and methods of manufacture

    SciTech Connect

    Torres, Ricardo D.; Sexton, Lindsay T.; Fuentes, Roderick E.; Cortes-Concepcion, Jose

    2015-08-11

    Photonic crystal scintillators and their methods of manufacture are provided. Exemplary methods of manufacture include using a highly-ordered porous anodic alumina membrane as a pattern transfer mask for either the etching of underlying material or for the deposition of additional material onto the surface of a scintillator. Exemplary detectors utilizing such photonic crystal scintillators are also provided.

  7. Neutron detection with single crystal organic scintillators

    SciTech Connect

    Zaitseva, N; Newby, J; Hamel, S; Carman, L; Faust, M; Lordi, V; Cherepy, N; Stoeffl, W; Payne, S

    2009-07-15

    Detection of high-energy neutrons in the presence of gamma radiation background utilizes pulse-shape discrimination (PSD) phenomena in organics studied previously only with limited number of materials, mostly liquid scintillators and single crystal stilbene. The current paper presents the results obtained with broader varieties of luminescent organic single crystals. The studies involve experimental tools of crystal growth and material characterization in combination with the advanced computer modeling, with the final goal of better understanding the relevance between the nature of the organic materials and their PSD properties. Special consideration is given to the factors that may diminish or even completely obscure the PSD properties in scintillating crystals. Among such factors are molecular and crystallographic structures that determine exchange coupling and exciton mobility in organic materials and the impurity effect discussed on the examples of trans-stilbene, bibenzyl, 9,10-diphenylanthracene and diphenylacetylene.

  8. Characterization of PbWO4 crystals for high-energy physics experiments

    NASA Astrophysics Data System (ADS)

    Kim, M. J.; Park, H.; Kim, H. J.

    2016-09-01

    High-energy physics (HEP) experiments have employed many new types of scintillators. Specifically, bismuth germanate, thallium-doped cesium iodide, and lead tungstate (PbWO4, PWO) have been used for the L3 experiment; CLEO II, Belle and BES-III; and CMS, respectively. PWO has particularly beneficial properties, such as high density, fast decay time, short radiation length and radiation hardness. In this study, we tested the PWO crystals at low temperatures to determine their applicability in future calorimeters. Various crystals from the Proton Antiproton Annihilations at Darmstadt (PANDA) experiment in Giessen, the Bogoroditsk Techno-Chemical Plant (BTCP) in Russia and by Shanghai Institute of Ceramics, Chinese Academy of Sciences (SICCAS) in China were investigated. We studied the scintillation properties of PWO crystals, such as their X-ray luminescence, relative light yields, absolute light yields, energy resolutions, decay times and longitudinal uniformities of their light yields. In addition, we measured the temperature dependences of the light yields and decay times by using a 137Cs γ-ray source. The emission spectra of the PWO crystals consisted of a broad band from 350 nm to 700 nm, and the peak emission wavelength in each spectrum was 420 nm. The emission spectra of the PWO crystals from SICCAS were slightly shifted to longer wavelengths compared with those of the crystals from the other institutions.

  9. New Scintillating Crystals for PET Scanners

    NASA Astrophysics Data System (ADS)

    Lecoq, Paul

    2002-01-01

    Systematic R&D on basic mechanism in inorganic scintillators, initiated by the Crystal Clear Collaboration at CERN 10 years ago, has contributed not to a small amount, to the development of new materials for a new generation of medical imaging devices with increased resolution and sensitivity. The first important requirement for a scintillator to be used in medical imaging devices is the stopping power for the given energy range of X and γ rays to be considered, and more precisely the conversion efficiency. A high light yield is also mandatory to improve the energy resolution, which is essentially limited by the photostatistics and the electronic noise at these energies. A short scintillation decay time allows to reduce the dead time and therefore to increase the limiting counting rate. When all these requirements are fulfilled the sensitivity and image contrast are increased for a given patient dose, or the dose can be reduced. Examples of new materials under development by the Crystal Clear Collaboration will be given with an emphasis on the major breakthrough they can bring in medical imaging, as compared to present equipments.

  10. Barium iodide single-crystal scintillator detectors

    NASA Astrophysics Data System (ADS)

    Cherepy, Nerine J.; Hull, Giulia; Niedermayr, Thomas R.; Drobshoff, Alexander; Payne, Stephen A.; Roy, Utpal N.; Cui, Yunlong; Bhattacharaya, Ajanta; Harrison, Melissa; Guo, Mingsheng; Groza, Michael; Burger, Arnold

    2007-09-01

    We find that the high-Z crystal Barium Iodide is readily growable by the Bridgman growth technique and is less prone to crack compared to Lanthanum Halides. We have grown Barium Iodide crystals: undoped, doped with Ce 3+, and doped with Eu 2+. Radioluminescence spectra and time-resolved decay were measured. BaI II(Eu) exhibits luminescence from both Eu 2+ at 420 nm (~450 ns decay), and a broad band at 550 nm (~3 μs decay) that we assign to a trapped exciton. The 550 nm luminescence decreases relative to the Eu 2+ luminescence when the Barium Iodide is zone refined prior to crystal growth. We also describe the performance of BaI II(Eu) crystals in experimental scintillator detectors.

  11. Crystal growth and scintillation properties of strontium iodide scintillators

    SciTech Connect

    van Loef, Edgar; Wilson, Cody; Cherepy, Nerine; Payne, Steven; Choong, Woon-Seng; Moses, William W.; Shah, Kanai

    2009-06-01

    Single crystals of SrI{sub 2}:Eu and SrI{sub 2}:Ce/Na were grown from anhydrous iodides by the vertical Bridgman technique in evacuated silica ampoules. Growth rates were of the order of 5-30 mm/day. Radioluminescence spectra of SrI{sub 2}:Eu and SrI{sub 2}:Ce/Na exhibit a broad band due to Eu{sup 2+} and Ce{sup 3+} emission, respectively. The maximum in the luminescence spectrum of SrI{sub 2}:Eu is found at 435 nm. The spectrum of SrI{sub 2}:Ce/Na exhibits a doublet peaking at 404 and 435 nm attributed to Ce{sup 3+} emission, while additional impurity - or defected - related emission is present at approximately 525 nm. The strontium iodide scintillators show very high light yields of up to 120,000 photons/MeV, have energy resolutions down to 3% at 662 keV (Full Width Half Maximum) and exhibit excellent light yield proportionality with a standard deviation of less than 5% between 6 and 460 keV.

  12. Scintillation of Un-doped ZnO Single Crystals

    SciTech Connect

    Colosimo, A. M.; Ji, Jianfeng; Stepanov, P. S.; Boatner, L. A.; Selim, F. A.

    2016-01-07

    In this paper, scintillation properties are often studied by photo-luminescence (PL) and scintillation measurements. In this work, we combine X-ray-induced luminescence (XRIL) spectroscopy [Review of Scientific Instruments 83, 103112 (2012)] with PL and standard scintillation measurements to give insight into the scintillation properties of un-doped ZnO single crystals. XRIL revealed that ZnO luminescence proportionally increases with X-ray power and exhibits excellent linearity - indicating the possibility of developing radiation detectors with good energy resolution. Finally, by coupling ZnO crystals to fast photomultiplier tubes and monitoring the anode signal, rise times as fast as 0.9 ns were measured.

  13. Divalent europium doped and un-doped calcium iodide scintillators: Scintillator characterization and single crystal growth

    DOE PAGES

    Boatner, L. A.; Ramey, J. O.; Kolopus, J. A.; ...

    2015-02-21

    Initially, the alkaline-earth scintillator, CaI2:Eu2+, was discovered around 1964 by Hofstadter, Odell, and Schmidt. Serious practical problems quickly arose, however, that were associated with the growth of large monolithic single crystals of this material due to its lamellar, mica-like structure. As a result of its theoretically higher light yield, CaI2:Eu2+ has the potential to exceed the excellent scintillation performance of SrI2:Eu2+. In fact, theoretical predictions for the light yield of CaI2:Eu2+ scintillators suggested that an energy resolution approaching 2% at 662 keV could be achievable. Like the early SrI2:Eu2+ scintillator, the performance of CaI2:Eu2+ scintillators has traditionally suffered due, atmore » least in part, to outdated materials synthesis, component stoichiometry/purity, and single-crystal-growth techniques. Based on our recent work on SrI2:Eu2+ scintillators in single-crystal form, we have developed new techniques that are applied here to CaI2:Eu2+ and pure CaI2 with the goal of growing large un-cracked crystals and, potentially, realizing the theoretically predicted performance of the CaI2:Eu2+ form of this material. Calcium iodide does not adhere to modern glassy carbon Bridgman crucibles - so there should be no differential thermal-contraction-induced crystal/crucible stresses on cooling that would result in crystal cracking of the lamellar structure of CaI2. Here we apply glassy carbon crucible Bridgman growth, high-purity growth-charge compounds, our molten salt processing/filtration technique, and extended vacuum-melt-pumping methods to the growth of both CaI2:Eu2+ and un-doped CaI2. Moreover, large scintillating single crystals were obtained, and detailed characterization studies of the scintillation properties of CaI2:Eu2+ and pure CaI2 single crystals are presented that include studies of the effects of plastic deformation of the crystals on the scintillator performance.« less

  14. Divalent europium doped and un-doped calcium iodide scintillators: Scintillator characterization and single crystal growth

    SciTech Connect

    Boatner, L. A.; Ramey, J. O.; Kolopus, J. A.; Neal, John S.

    2015-02-21

    Initially, the alkaline-earth scintillator, CaI2:Eu2+, was discovered around 1964 by Hofstadter, Odell, and Schmidt. Serious practical problems quickly arose, however, that were associated with the growth of large monolithic single crystals of this material due to its lamellar, mica-like structure. As a result of its theoretically higher light yield, CaI2:Eu2+ has the potential to exceed the excellent scintillation performance of SrI2:Eu2+. In fact, theoretical predictions for the light yield of CaI2:Eu2+ scintillators suggested that an energy resolution approaching 2% at 662 keV could be achievable. Like the early SrI2:Eu2+ scintillator, the performance of CaI2:Eu2+ scintillators has traditionally suffered due, at least in part, to outdated materials synthesis, component stoichiometry/purity, and single-crystal-growth techniques. Based on our recent work on SrI2:Eu2+ scintillators in single-crystal form, we have developed new techniques that are applied here to CaI2:Eu2+ and pure CaI2 with the goal of growing large un-cracked crystals and, potentially, realizing the theoretically predicted performance of the CaI2:Eu2+ form of this material. Calcium iodide does not adhere to modern glassy carbon Bridgman crucibles - so there should be no differential thermal-contraction-induced crystal/crucible stresses on cooling that would result in crystal cracking of the lamellar structure of CaI2. Here we apply glassy carbon crucible Bridgman growth, high-purity growth-charge compounds, our molten salt processing/filtration technique, and extended vacuum-melt-pumping methods to the growth of both CaI2:Eu2+ and un-doped CaI2. Moreover, large scintillating single crystals were obtained, and detailed characterization studies of the

  15. Visible scintillation photodetector device incorporating chalcopyrite semiconductor crystals

    DOEpatents

    Stowe, Ashley C.; Burger, Arnold

    2017-04-04

    A photodetector device, including: a scintillator material operable for receiving incident radiation and emitting photons in response; a photodetector material coupled to the scintillator material operable for receiving the photons emitted by the scintillator material and generating a current in response, wherein the photodetector material includes a chalcopyrite semiconductor crystal; and a circuit coupled to the photodetector material operable for characterizing the incident radiation based on the current generated by the photodetector material. Optionally, the scintillator material includes a gamma scintillator material and the incident radiation received includes gamma rays. Optionally, the photodetector material is further operable for receiving thermal neutrons and generating a current in response. The circuit is further operable for characterizing the thermal neutrons based on the current generated by the photodetector material.

  16. Event localization in bulk scintillator crystals using coded apertures

    NASA Astrophysics Data System (ADS)

    Ziock, K. P.; Braverman, J. B.; Fabris, L.; Harrison, M. J.; Hornback, D.; Newby, J.

    2015-06-01

    The localization of radiation interactions in bulk scintillators is generally limited by the size of the light distribution at the readout surface of the crystal/light-pipe system. By finding the centroid of the light spot, which is typically of order centimeters across, practical single-event localization is limited to 2 mm/cm of crystal thickness. Similar resolution can also be achieved for the depth of interaction by measuring the size of the light spot. Through the use of near-field coded-aperture techniques applied to the scintillation light, light transport simulations show that for 3-cm-thick crystals, more than a five-fold improvement (millimeter spatial resolution) can be achieved both laterally and in event depth. At the core of the technique is the requirement to resolve the shadow from an optical mask placed in the scintillation light path between the crystal and the readout. In this paper, experimental results are presented that demonstrate the overall concept using a 1D shadow mask, a thin-scintillator crystal and a light pipe of varying thickness to emulate a 2.2-cm-thick crystal. Spatial resolutions of 1 mm in both depth and transverse to the readout face are obtained over most of the crystal depth.

  17. Event Localization in Bulk Scintillator Crystals Using Coded Apertures

    SciTech Connect

    Ziock, Klaus-Peter; Braverman, Joshua B.; Fabris, Lorenzo; Harrison, Mark J.; Hornback, Donald Eric; Newby, Jason

    2015-06-01

    The localization of radiation interactions in bulk scintillators is generally limited by the size of the light distribution at the readout surface of the crystal/light-pipe system. By finding the centroid of the light spot, which is typically of order centimeters across, practical single-event localization is limited to ~2 mm/cm of crystal thickness. Similar resolution can also be achieved for the depth of interaction by measuring the size of the light spot. Through the use of near-field coded-aperture techniques applied to the scintillation light, light transport simulations show that for 3-cm-thick crystals, more than a five-fold improvement (millimeter spatial resolution) can be achieved both laterally and in event depth. At the core of the technique is the requirement to resolve the shadow from an optical mask placed in the scintillation light path between the crystal and the readout. In this paper, experimental results are presented that demonstrate the overall concept using a 1D shadow mask, a thin-scintillator crystal and a light pipe of varying thickness to emulate a 2.2-cm-thick crystal. Spatial resolutions of ~ 1 mm in both depth and transverse to the readout face are obtained over most of the crystal depth.

  18. X-ray Scintillation in Lead Halide Perovskite Crystals

    PubMed Central

    Birowosuto, M. D.; Cortecchia, D.; Drozdowski, W.; Brylew, K.; Lachmanski, W.; Bruno, A.; Soci, C.

    2016-01-01

    Current technologies for X-ray detection rely on scintillation from expensive inorganic crystals grown at high-temperature, which so far has hindered the development of large-area scintillator arrays. Thanks to the presence of heavy atoms, solution-grown hybrid lead halide perovskite single crystals exhibit short X-ray absorption length and excellent detection efficiency. Here we compare X-ray scintillator characteristics of three-dimensional (3D) MAPbI3 and MAPbBr3 and two-dimensional (2D) (EDBE)PbCl4 hybrid perovskite crystals. X-ray excited thermoluminescence measurements indicate the absence of deep traps and a very small density of shallow trap states, which lessens after-glow effects. All perovskite single crystals exhibit high X-ray excited luminescence yields of >120,000 photons/MeV at low temperature. Although thermal quenching is significant at room temperature, the large exciton binding energy of 2D (EDBE)PbCl4 significantly reduces thermal effects compared to 3D perovskites, and moderate light yield of 9,000 photons/MeV can be achieved even at room temperature. This highlights the potential of 2D metal halide perovskites for large-area and low-cost scintillator devices for medical, security and scientific applications. PMID:27849019

  19. X-ray Scintillation in Lead Halide Perovskite Crystals

    NASA Astrophysics Data System (ADS)

    Birowosuto, M. D.; Cortecchia, D.; Drozdowski, W.; Brylew, K.; Lachmanski, W.; Bruno, A.; Soci, C.

    2016-11-01

    Current technologies for X-ray detection rely on scintillation from expensive inorganic crystals grown at high-temperature, which so far has hindered the development of large-area scintillator arrays. Thanks to the presence of heavy atoms, solution-grown hybrid lead halide perovskite single crystals exhibit short X-ray absorption length and excellent detection efficiency. Here we compare X-ray scintillator characteristics of three-dimensional (3D) MAPbI3 and MAPbBr3 and two-dimensional (2D) (EDBE)PbCl4 hybrid perovskite crystals. X-ray excited thermoluminescence measurements indicate the absence of deep traps and a very small density of shallow trap states, which lessens after-glow effects. All perovskite single crystals exhibit high X-ray excited luminescence yields of >120,000 photons/MeV at low temperature. Although thermal quenching is significant at room temperature, the large exciton binding energy of 2D (EDBE)PbCl4 significantly reduces thermal effects compared to 3D perovskites, and moderate light yield of 9,000 photons/MeV can be achieved even at room temperature. This highlights the potential of 2D metal halide perovskites for large-area and low-cost scintillator devices for medical, security and scientific applications.

  20. An analysis of side readouts of monolithic scintillation crystals

    NASA Astrophysics Data System (ADS)

    Li, Xin; Furenlid, Lars R.

    2016-10-01

    We have explored a method of using the side surfaces of a thin monolithic scintillation crystal for reading out scintillation photons. A Monte-Carlo simulation was carried out for an LYSO crystal of 50:8mmx50:8mmx3mm with 5 silicon photomultipliers attached on each of the four side surfaces. With 511 keV gamma-rays, X-Y spatial resolution of 2:10mm was predicted with an energy resolution of 9:0%. We also explored adding optical barriers to improve the X-Y spatial resolution, and an X-Y spatial resolution of 786um was predicted with an energy resolution of 9:2%. Multiple layers can be stacked together and readout channels can be combined. Depth-of- interaction information (DOI) can be directly read out. This method provides an attractive detector module design for positron emission tomography (PET).

  1. Improving scintillation crystals using muon tomography

    SciTech Connect

    Dowell, D.H.; Fineman, B.J.; Sandorfi, A.M.

    1987-01-01

    The cosmic ray muon scanning array provides information on NaI(T1) crystals using some 65,536 trajectories, each measuring the NaI(T1) response to high energy muons. With this information, it is possible to use established computer-aided-tomography techniques to deconvolute these integrated responses and produce a detailed picture of the detector's interior.

  2. Free carrier absorption in self-activated PbWO4 and Ce-doped Y3(Al0.25Ga0.75)3O12 and Gd3Al2Ga3O12 garnet scintillators

    NASA Astrophysics Data System (ADS)

    Auffray, E.; Korjik, M.; Lucchini, M. T.; Nargelas, S.; Sidletskiy, O.; Tamulaitis, G.; Tratsiak, Y.; Vaitkevičius, A.

    2016-08-01

    Nonequilibrium carrier dynamics in the scintillators prospective for fast timing in high energy physics and medical imaging applications was studied. The time-resolved free carrier absorption investigation was carried out to study the dynamics of nonequilibrium carriers in wide-band-gap scintillation materials: self-activated led tungstate (PbWO4, PWO) ant two garnet crystals, GAGG:Ce and YAGG:Ce. It was shown that free electrons appear in the conduction band of PWO and YAGG:Ce crystals within a sub-picosecond time scale, while the free holes in GAGG:Ce appear due to delocalization from Gd3+ ground states to the valence band within a few picoseconds after short-pulse excitation. The influence of Gd ions on the nonequilibrium carrier dynamics is discussed on the base of comparison the results of the free carrier absorption in GAGG:Ce containing gadolinium and in YAGG without Gd in the host lattice.

  3. Barium iodide and strontium iodide crystals andd scintillators implementing the same

    SciTech Connect

    Payne, Stephen A; Cherepy, Nerine J; Hull, Giulia E; Drobshoff, Alexander D; Burger, Arnold

    2013-11-12

    In one embodiment, a material comprises a crystal comprising strontium iodide providing at least 50,000 photons per MeV. A scintillator radiation detector according to another embodiment includes a scintillator optic comprising europium-doped strontium iodide providing at least 50,000 photons per MeV. A scintillator radiation detector in yet another embodiment includes a scintillator optic comprising SrI.sub.2 and BaI.sub.2, wherein a ratio of SrI.sub.2 to BaI.sub.2 is in a range of between 0:1 A method for manufacturing a crystal suitable for use in a scintillator includes mixing strontium iodide-containing crystals with a source of Eu.sup.2+, heating the mixture above a melting point of the strontium iodide-containing crystals, and cooling the heated mixture near the seed crystal for growing a crystal. Additional materials, systems, and methods are presented.

  4. Effects of Packaging SrI2(Eu) Scintillator Crystals

    SciTech Connect

    Sturm, Benjamin; Cherepy, Nerine; Drury, Owen; Thelin, P; Fisher, S E; Payne, Stephen A.; Burger, Arnold; Boatner, Lynn A; Ramey, Joanne Oxendine; Shah, Kanai; Hawrami, Rastgo

    2011-01-01

    Recent renewed emphasis placed on gamma-ray detectors for national security purposes has motivated 13 researchers to identify and develop new scintillator materials capable of high energy resolution and 14 growable to large sizes. We have discovered that SrI2(Eu) has many desirable properties for gamma-ray 15 detection and spectroscopy, including high light yield of ~90,000 photons/MeV and excellent light yield 16 proportionality. Furthermore, we have demonstrated growth of crack-free 2 diameter boules. We 17 have measured <2.7% FWHM at 662 keV with small detectors (<1 cm3) in direct contact with a 18 photomultiplier tube, and ~3% resolution at 662 keV is obtained for 1 in3 crystals. Due to the 19 hygroscopic nature of SrI2(Eu), proper packaging is required for field use. This work describes a 20 systematic study performed to determine the key factors in the packaging process to optimize 21 performance. These factors include proper polishing of the surface, the geometry of the crystal, 22 reflector materials and windows. A technique based on use of a collimated Cs-137 source was developed 23 to examine light collection uniformity. Employing this technique, we found that when the crystal is 24 packaged properly, the variance in the pulse height at 662 keV from events near the bottom of the 25 crystal compared to those near the top of the crystal could be reduced to <1%. This paper describes the 26 design and engineering of our detector package in order to improve energy resolution of 1 in3-scale 27 SrI2(Eu) crystals.

  5. Scintillation properties of SrF2 and SrF2-Ce3+ crystals

    NASA Astrophysics Data System (ADS)

    Shendrik, R. Yu.; Radzhabov, E. A.; Nepomnyashchikh, A. I.

    2013-07-01

    This Letter presents the results of measuring scintillation properties of pure SrF2 crystals and crystals activated by various concentrations of Ce3+ ions. The light yield of these materials is compared to that of the known scintillators NaI-Tl and CaF2-Eu2+. Strontium fluoride crystals activated with Ce3+ ions are found to be characterized by high light yield and to be promising materials for use in scintillation detectors employed for γ-ray well logging.

  6. Crystal growth and scintillation properties of Lu substituted CeBr3 single crystals

    NASA Astrophysics Data System (ADS)

    Ito, Tomoki; Yokota, Yuui; Kurosawa, Shunsuke; Král, Robert; Kamada, Kei; Pejchal, Jan; Ohashi, Yuji; Yoshikawa, Akira

    2016-10-01

    We grew Lu-substituted CeBr3 [(Ce1-xLux)Br3] crystals by a modified micro-pulling-down method to increase the effective atomic number and to investigate effects of the Lu substitution on the crystal growth, phase generation, chemical composition, and optical and scintillation properties. The (Ce1-xLux)Br3 crystals with x=0 and 0.01 had high transparency while the milky parts were generated in the crystals with x=0.05 and 0.20. By the analysis of chemical composition, the estimated Zeff increased to 47.9. On the other hand, the light yields were systematically decreased and decay times were increased with increasing Lu concentration.

  7. A crystal identification method for monolithic phoswich detectors based on scintillation light distribution

    NASA Astrophysics Data System (ADS)

    Preziosi, E.; Pani, R.; Trigila, C.; Polito, C.; Bettiol, M.; Borrazzo, C.; Cinti, M. N.; Fabbri, A.; Pellegrini, R.; Pani, R.

    2016-12-01

    Phoswich detectors based on scintillation crystals are widely diffused for both PET and SPECT applications. In order to separate the signals arising from different layers many methods have been proposed in literature. Separation of the layers commonly relies on time discrimination or pulse height discrimination. In this work, by means of experimental measurement on a phoswich detector based on Lanthanum Bromide and Lutetium Fine Silicate monolithic crystals, a novel method allowing to separate signals coming from different layers has been evaluated. The main feature of this method, specifically developed for phoswich based on monolithic scintillation crystals, is the discrimination capability based on the scintillation light distribution shape. For this reason, the findings that will be shown could be easily extended to whatever combination of scintillator, independently from their decay time or light yield.

  8. Barium iodide and strontium iodide crystals and scintillators implementing the same

    DOEpatents

    Payne, Stephen A.; Cherepy, Nerine J.; Hull, Giulia E.; Drobshoff, Alexander D.; Burger, Arnold

    2016-11-29

    In one embodiment, a material comprises a crystal comprising strontium iodide providing at least 50,000 photons per MeV, where the strontium iodide material is characterized by a volume not less than 1 cm.sup.3. In another embodiment, a scintillator optic includes europium-doped strontium iodide providing at least 50,000 photons per MeV, where the europium in the crystal is primarily Eu.sup.2+, and the europium is present in an amount greater than about 1.6%. A scintillator radiation detector in yet another embodiment includes a scintillator optic comprising SrI.sub.2 and BaI.sub.2, where a ratio of SrI.sub.2 to BaI.sub.2 is in a range of between 0:1 and 1.0, the scintillator optic is a crystal that provides at least 50,000 scintillation photons per MeV and energy resolution of less than about 5% at 662 keV, and the crystal has a volume of 1 cm.sup.3 or more; the scintillator optic contains more than about 2% europium.

  9. Characterization of BaCl 2 scintillation crystal at low temperature

    NASA Astrophysics Data System (ADS)

    Kim, M. J.; Kim, H. J.; Park, H.; Kim, Sunghwan; Kim, Jung-in

    2011-03-01

    A BaCl 2 scintillation crystal was grown by the Czochralski method. The grown crystal was cut to a size of 10×10×5 mm 3. The scintillation properties of the crystal such as pulse height spectra, energy resolution, and fluorescence decay time were measured with a 137Cs (662 keV) γ-ray source at room temperature. We measured the temperature dependence of the scintillation light yield and decay time with a bi-alkali photomultiplier tube for the BaCl 2 crystal. The BaCl 2 crystal was cooled down with compressed helium gas from room temperature to 10 K. We measured the light yield and decay time changes of the BaCl 2 crystal from 10 K to room temperature. The light yield of the BaCl 2 at 200 K was four times higher than that at room temperature. The decay time increases as temperature decreases. The BaCl 2 scintillation crystal has a low light yield but a fast decay time so that it can be a calorimeter candidate for high energy physics experiments.

  10. Comparative study of intrinsic luminescence in undoped transparent ceramic and single crystal garnet scintillators

    NASA Astrophysics Data System (ADS)

    Fujimoto, Yutaka; Yanagida, Takayuki; Yagi, Hideki; Yanagidani, Takagimi; Chani, Valery

    2014-10-01

    Scintillation properties associated with intrinsic lattice defects of undoped Y3A5O12 (YAG) and Lu3A5O12 (LuAG) transparent ceramics and single crystals are compared. The ceramics excited with X-ray demonstrated relatively low emission intensity when compared with that of the single crystals. Decay times of the ceramics and the single crystals were similar. These parameters were approximately 430 ns (YAG ceramic), 460 ns (YAG single crystal), 30 ns and 1090 ns (LuAG ceramic), and 25 ns and 970 ns (LuAG single crystal). According to the pulse height spectra recorded under 137Cs gamma-ray irradiation, the scintillation light yield of the both ceramics were about 2950 ± 290 ph/MeV. However, the single crystals had greater kight yield of about about 14,300 ± 1430 ph/MeV for YAG and 8350 ± 830 ph/MeV for LuAG.

  11. Study of the growth atmosphere effect on optical and scintillation characteristics of large CsI(TI) crystals

    NASA Astrophysics Data System (ADS)

    Panova, A. N.; Goriletsky, V. I.; Grinyova, T. B.; Shakhova, K. V.; Vinograd, E. L.

    1999-03-01

    In contrast to the traditional growth method of large scintillation alkali halide crystals - in an inert atmosphere, CsI(TI) crystals have been grown in CO 2 atmosphere favoring changes of their impurity composition. Absorption and scintillation characteristics of crystals obtained have been studied in comparison to those grown in the inert gas medium. Effect of different radiation doses on variations in optical and scintillation characteristics has been studied for CsI(TI) crystals grown by various techniques. CsI(TI) crystals grown in CO 2 atmosphere are found to exhibit a higher radiation resistance and a faster restoration of their basic characteristics.

  12. Modified timing characteristic of a scintillation detection system with photonic crystal structures.

    PubMed

    Liu, Jinliang; Liu, Bo; Zhu, Zhichao; Chen, Liang; Hu, Jing; Xu, Mengxuan; Cheng, Chuanwei; Ouyang, Xiaoping; Zhang, Zhongbing; Ruan, Jinlu; He, Shiyi; Liu, Linyue; Gu, Mu; Chen, Hong

    2017-03-01

    It is intuitively expected that an enhanced light extraction of a scintillator can be easily achieved by photonic crystal structures. Here, we demonstrate a modified timing characteristic for a detection system induced by enhanced light extraction with photonic crystal structures. Such improvement is due to the enhanced light extraction which can be clearly proven by the independent measurements of the light output and the timing resolution. The present investigation is advantageous to promote the development of a scintillation detection system performance based on the time-of-flight measurement.

  13. Fast ultradense GdTa1-xNbxO4 scintillator crystals

    NASA Astrophysics Data System (ADS)

    Voloshyna, Olesia; Gerasymov, Iaroslav; Sidletskiy, Oleg; Kurtsev, Daniil; Gorbacheva, Tatyana; Hubenko, Kateryna; Boiaryntseva, Ianina; Ivanov, Alexey; Spassky, Dmitry; Omelkov, Sergey; Belsky, Andrei

    2017-04-01

    Single crystals of GdTaO4 and GdTa0.8Nb0.2O4 were grown by the Czochralski technique, and their luminescent and scintillation properties were studied. Both crystals demonstrate fast emission with decay time around 10-8 s. Meanwhile, in GdTaO4 the fast decay is accompanied by a huge build-up with the decay time around 1 μs, while in the mixed crystal the contribution of slow components is negligible. UV- and X-ray excited luminescence, curves of thermostimulated luminescence and absolute light yields of crystals are presented as well. GdTa0.8Nb0.2O4 crystal is shown to be an ultradense (8.37 g/cm3) and fast (shortest component decay time 17 ns) scintillator with a high stopping power.

  14. Formation of light-reflecting powder shells for scintillation crystals with a complicated shape

    SciTech Connect

    Mel`nik, V.I.; Grinev, B.V.

    1995-10-01

    Technical means for mechanized formation of light-reflecting powder shells of scintillation crystals with a complicated shape that is close to conical are unknown at present. Below, we suggest a design for such technical facilities, a technology for assembling detectors with their aid, and the selection of the operational parameters of the assembly.

  15. Defect Engineering in SrI2:Eu2+ Single Crystal Scintillators

    DOE PAGES

    Wu, Yuntao; Boatner, Lynn A.; Lindsey, Adam C.; ...

    2015-06-23

    Eu2+-activated strontium iodide is an excellent single crystal scintillator used for gamma-ray detection and significant effort is currently focused on the development of large-scale crystal growth techniques. A new approach of molten-salt pumping or so-called melt aging was recently applied to optimize the crystal quality and scintillation performance. Nevertheless, a detailed understanding of the underlying mechanism of this technique is still lacking. The main purpose of this paper is to conduct an in-depth study of the interplay between microstructure, trap centers and scintillation efficiency after melt aging treatment. Three SrI2:2 mol% Eu2+ single crystals with 16 mm diameter were grownmore » using the Bridgman method under identical growth conditions with the exception of the melt aging time (e.g. 0, 24 and 72 hours). Using energy-dispersive X-ray spectroscopy, it is found that the matrix composition of the finished crystal after melt aging treatment approaches the stoichiometric composition. The mechanism responsible for the formation of secondary phase inclusions in melt-aged SrI2:Eu2+ is discussed. Simultaneous improvement in light yield, energy resolution, scintillation decay-time and afterglow is achieved in melt-aged SrI2:Eu2+. The correlation between performance improvement and defect structure is addressed. The results of this paper lead to a better understanding of the effects of defect engineering in control and optimization of metal halide scintillators using the melt aging technique.« less

  16. Cesium hafnium chloride: A high light yield, non-hygroscopic cubic crystal scintillator for gamma spectroscopy

    SciTech Connect

    Burger, Arnold; Rowe, Emmanuel; Groza, Michael; Morales Figueroa, Kristle; Cherepy, Nerine J.; Beck, Patrick R.; Hunter, Steven; Payne, Stephen A.

    2015-10-05

    We report on the scintillation properties of Cs{sub 2}HfCl{sub 6} (cesium hafnium chloride or CHC) as an example of a little-known class of non-hygroscopic compounds having the generic cubic crystal structure of K{sub 2}PtCl{sub 6}. The crystals are easily growable from the melt using the Bridgman method with minimal precursor treatments or purification. CHC scintillation is centered at 400 nm, with a principal decay time of 4.37 μs and a light yield of up to 54 000 photons/MeV when measured using a silicon CCD photodetector. The light yield is the highest ever reported for an undoped crystal, and CHC also exhibits excellent light yield nonproportionality. These desirable properties allowed us to build and test CHC gamma-ray spectrometers providing energy resolution of 3.3% at 662 keV.

  17. R and D of crystal scintillators from enriched isotopes for high sensitivity double β decay experiments

    SciTech Connect

    Danevich, F. A.

    2013-12-30

    Experiments to search for neutrinoless double beta decay enters to a new phase when a sensitivity on the level of T{sub 1/2}∼10{sup 26}−10{sup 28} yr is required. Scintillating low temperature detectors possess important properties required for high-sensitivity double beta decay experiments: presence of elements of interest, high energy resolution and detection efficiency, low level of background thanks to excellent particle discrimination ability. High concentration of isotope of interest and as low as possible radioactive contamination are important requirements to crystal scintillators. Other crucial issues are maximal output of detectors and minimal loss of enriched materials. Prospects of several scintillation materials, enriched in isotopes promising for double beta decay experiments, are discussed.

  18. Advances in the growth of alkaline-earth halide single crystals for scintillator detectors

    SciTech Connect

    Boatner, Lynn A; Ramey, Joanne Oxendine; Kolopus, James A; Neal, John S; Cherepy, Nerine; Payne, Stephen A.; Beck, P; Burger, Arnold; Rowe, E; Bhattacharya, P.

    2014-01-01

    Alkaline-earth scintillators such as strontium iodide and other alkaline-earth halides activated with divalent europium represent some of the most efficient and highest energy resolution scintillators for use as gamma-ray detectors in a wide range of applications. These applications include the areas of nuclear nonproliferation, homeland security, the detection of undeclared nuclear material, nuclear physics and materials science, medical diagnostics, space physics, high energy physics, and radiation monitoring systems for first responders, police, and fire/rescue personnel. Recent advances in the growth of large single crystals of these scintillator materials hold the promise of higher crystal yields and significantly lower detector production costs. In the present work, we describe new processing protocols that, when combined with our molten salt filtration methods, have led to advances in achieving a significant reduction of cracking effects during the growth of single crystals of SrI2:Eu2+. In particular, we have found that extended pumping on the molten crystal-growth charge under vacuum for time periods extending up to 48 hours is generally beneficial in compensating for variations in the alkaline-earth halide purity and stoichiometry of the materials as initially supplied by commercial sources. These melt-pumping and processing techniques are now being applied to the purification of CaI2:Eu2+ and some mixed-anion europium-doped alkaline-earth halides prior to single-crystal growth by means of the vertical Bridgman technique. The results of initial studies of the effects of aliovalent doping of SrI2:Eu2+ on the scintillation characteristics of this material are also described.

  19. Investigation of the unique degradation phenomenon observed in CsSrBr3: Eu 5% scintillator crystals

    NASA Astrophysics Data System (ADS)

    Gokhale, S. S.; Loyd, M.; Stand, L.; Lindsey, A.; Swider, S.; Zhuravleva, M.; Melcher, C. L.

    2016-10-01

    CsSrBr3: Eu 5% is a promising compound scintillator for radiation detection and imaging applications. Light output and energy resolution measured for a crystal of volume 5×5×5 mm3 were 55,000±2000 ph/MeV and 5.6% at 662 keV respectively which is a significant improvement over previous reports. The hygroscopicity of the compound and the tendency of the scintillator crystals to degrade when exposed to the atmosphere necessitate the proper encapsulation of the crystals. It was observed that unlike other hygroscopic scintillator crystals CsSrBr3 undergoes a unique degradation while encapsulated in mineral oil. The light output of the crystal decreases over time, but there is no visually observed physical degradation of the crystal. This degradation is a reversible process wherein a degraded crystal can be subjected to annealing in vacuum in order to restore its original performance.

  20. Crystal growth and scintillation properties of undoped and Ce3+-doped GdI3 crystals

    NASA Astrophysics Data System (ADS)

    Ye, Le; Li, Huanying; Wang, Chao; Shi, Jian; Chen, Xiaofeng; Wang, Zhongqing; Huang, Yuefeng; Xu, Jiayue; Ren, Guohao

    2017-02-01

    The growth and scintillation properties of undoped and Ce3+-doped GdI3 crystals were reported in this paper. These GdI3:χ%Ce (χ = 0, 1, 2) crystals were grown by the vertical Bridgman growth technique in evacuated quartz crucibles. X-ray excited optical luminescence spectra of GdI3:Ce exhibit a broad emission band (450 nm-650 nm) peaking at 520 nm corresponding to 5d1→4f1 transition of Ce3+ while the undoped GdI3 crystal consists of a broad band (400 nm-600 nm) and several sharp lines peaking at 462 nm, 482 nm, 492 nm, 549 nm, 579 nm owing to the impurities ions and defects. The excitation spectra of Ce3+ doped GdI3 consist of two broad bands between 300 nm and 500 nm corresponding to 4f1→5d1 absorption of Ce3+. The other absorption peaking at 262 nm in the spectrum of GdI3:2%Ce is assigned to band-to-band exciton transition. The excitation spectrum of undoped GdI3 contains a flat absorption band from 330 to 370 nm and a broad band between 390 and 450 nm peaking at 414 nm corresponding to the absorption of the unintentionally doped Ce3+, Dy3+, Ho3+ impurities and other defects. The emission spectrum of undoped GdI3 under 332 nm excitation has the identical line peaks with the spectrum measured under X-ray excitation. The emission spectra of GdI3:2%Ce and GdI3:1%Ce show a broad band in the range of 450-750 nm with the maximum at 550 nm corresponding to 5d1→4f1 transitions of Ce3+ ion. The GdI3, GdI3:1%Ce and GdI3:2%Ce show fast principle decay time constant 73 ns, 69 ns and 58 ns respectively, besides, the undoped also shows a slow decay constant 325 ns which doesn't appear in Ce3+-doped GdI3 crystal. The energy resolutions of GdI3:χ%Ce (χ = 1, 2) measured at 662 KeV are about 3%-5% and the undoped GdI3 is 13.3%.

  1. Barium iodide and strontium iodide crystals and scintillators implementing the same

    DOEpatents

    Payne, Stephen A.; Cherepy, Nerine; Pedrini, Christian; Burger, Arnold

    2016-09-13

    In one embodiment, a crystal includes at least one metal halide; and an activator dopant comprising ytterbium. In another general embodiment, a scintillator optic includes: at least one metal halide doped with a plurality of activators, the plurality of activators comprising: a first activator comprising europium, and a second activator comprising ytterbium. In yet another general embodiment, a method for manufacturing a crystal suitable for use in a scintillator includes mixing one or more salts with a source of at least one dopant activator comprising ytterbium; heating the mixture above a melting point of the salt(s); and cooling the heated mixture to a temperature below the melting point of the salts. Additional materials, systems, and methods are presented.

  2. Advances in the growth of alkaline-Earth halide single crystals for scintillator detectors

    NASA Astrophysics Data System (ADS)

    Boatner, L. A.; Ramey, J. O.; Kolopus, J. A.; Neal, J. S.; Cherepy, N. J.; Beck, P. R.; Payne, S. A.; Burger, A.; Rowe, E.; Bhattacharya, P.

    2014-09-01

    Alkaline-earth scintillators such as strontium iodide and other alkaline-earth halides activated with divalent europium represent some of the most efficient and highest energy resolution scintillators for use as gamma-ray detectors in a wide range of applications. These applications include the areas of nuclear nonproliferation, homeland security, the detection of undeclared nuclear material, nuclear physics and materials science, medical diagnostics, space physics, high energy physics, and radiation monitoring systems for first responders, police, and fire/rescue personnel. Recent advances in the growth of large single crystals of these scintillator materials hold the promise of higher crystal yields and significantly lower detector production costs. In the present work, we describe new processing protocols that, when combined with our molten salt filtration methods, have led to advances in achieving a significant reduction of cracking effects during the growth of single crystals of SrI2:Eu2+. In particular, we have found that extended pumping on the molten crystalgrowth charge under vacuum for time periods extending up to 48 hours is generally beneficial in compensating for variations in the alkaline-earth halide purity and stoichiometry of the materials as initially supplied by commercial sources. These melt-pumping and processing techniques are now being applied to the purification of CaI2:Eu2+ and some mixed-anion europium-doped alkaline-earth halides prior to single-crystal growth by means of the vertical Bridgman technique. The results of initial studies of the effects of aliovalent doping of SrI2:Eu2+ on the scintillation characteristics of this material are also described.

  3. The Characterization of Eu2+-Doped Mixed Alkaline-Earth Iodide Scintillator Crystals

    SciTech Connect

    Neal, John S; Boatner, Lynn A; Ramey, Joanne Oxendine; Wisniewski, D.; Kolopus, James A; Cherepy, Nerine; Payne, Stephen A.

    2011-01-01

    The high-performance inorganic scintillator, SrI2:Eu2+, when activated with divalent europium in the concentration range of 3 to 6%, has shown great promise for use in applications that require high-energy-resolution gamma-ray detection. We have recently grown and tested crystals in which other alkaline-earth ions have been partially substituted for Sr ions. Specifically, europium-doped single crystals have been grown in which up to 30 at % of the strontium ions have been substituted for either by barium, magnesium, or calcium ions. In the case of the strontium iodide scintillator host, a material that is characterized by an orthorhombic crystal structure, there are three other column IIA elements that are obvious choices for investigations whose purpose is to realize potential improvements in the performance of SrI2:Eu2+-based scintillators via the replacement of strontium ions with either Mg2+, Ca2+, or Ba2+. Light yields of up to 81,400 photons/MeV with an associated energy resolution of 3.7% (fwhm for 662 keV gamma-rays) have been observed in the case of a partial substitution of Ba2+ for Sr2+. The measured decay times ranged from 1.1 to 2.0 s, while the peak emission wavelengths ranged from 432 to 438 nm.

  4. Performance study of Philips digital silicon photomultiplier coupled to scintillating crystals

    NASA Astrophysics Data System (ADS)

    Liu, Z.; Pizzichemi, M.; Auffray, E.; Lecoq, P.; Paganoni, M.

    2016-01-01

    Silicon photomultipliers (SiPMs) and scintillators are often arranged in the shape of arrays in Positron Emission Tomography (PET) systems. Digital SiPMs provide signal readout in single photon avalanche diode (SPAD) level. From the photon count rate measurement of each SPAD cell of digital SiPM, we found that the output scintillating photons distribute in an area larger than the scintillator physical coupling area. Taking advantage of the possibility to enable/disable individual cells of the digital SiPM, a group of Lutetium-yttrium oxyorthosilicate (LYSO) crystals with different dimensions coupled to a digital SiPM was used to study the influence of using different SiPM active area on the number of photons detected, energy resolution and coincidence time resolution (CTR). For the same crystal coupled to the digital SiPM, the larger the active area of digital SiPM, the higher the number of photons detected. The larger active area of the digital SiPM also results in a better energy resolution after saturation correction. The best energy resolution full width half maximum (FWHM) obtained for the 2 × 2 × 5 mm3, 2 × 2 × 10 mm3, 2 × 2 × 15 mm3, 2 × 2 × 20 mm3 LYSO crystals was 10.7%, 11.6%, 12.1%, 12.5%, respectively. For crystals with different cross sections coupled to the digital SiPM, we found that the larger the cross section of coupling area, the more photons were detected and thus a better energy resolution was obtained. The CTR of crystals fully wrapped with Teflon or without wrapping was measured by positioning two identical crystals facing each other. A larger area of digital SiPM improves the CTR and the CTR reaches the plateau when the active area is larger than 2.2 × 2.2 mm2 with both two configurations of wrapping. The best CTR value for the 2 × 2 × 5 mm3, 2 × 2 × 10 mm3, 2 × 2 × 15 mm3, 2 × 2 × 20 mm3 LYSO crystals was 128.9 ps, 148.4 ps, 171.6 ps, 177.9 ps, respectively. The measurements performed lead us to conclude that optimising the

  5. Complex defects in crystal scintillation materials and phosphors

    NASA Astrophysics Data System (ADS)

    Lisitsyn, V.; Lisitsyna, L.; Polisadova, E.

    2017-01-01

    The possibility of the existence of complex defects in pure and doped crystal phosphor discussed in work. The luminescent properties of mono- and nanocrystals of zinc tungstate, the powders of YAG with various compositions are studied. It is shown that the intrinsic defects, impurities, oxygen vacancies, the hydroxyl groups may be present in the structure of the complex defects (nanodefects). Nanodefects form during synthesis and have high efficiency of the transfer of excitation energy to the emission centres.

  6. Ionization and proton induced radiation damage in crystal scintillators (Conference Presentation)

    NASA Astrophysics Data System (ADS)

    Zhu, Ren-Yuan

    2016-09-01

    Crystal detectors have been used widely in high energy and nuclear physics experiments, medical instruments and homeland security applications. A crucial issue for crystal detectors to be used for future HEP experiments at the energy and intensity frontiers is radiation damage by ionization dose as well as charged and neutral hadrons. This paper reports recent investigations on radiation damage in various crystal scintillators. Irradiations up to 340 Mrad of ionization dose, 1E16 p/cm^2 fluence and 1016 n/cm2 fluence were carried out at the JPL total ionization dose facility and the Los Alamos Neutron Science Center, respectively. Results of these investigations show excellent radiation hardness of bright and fast LYSO crystals which may provide a stable detector in an extreme harsh radiation environment, such as the proposed HL-LHC.

  7. Technical Scope of Work: Proton Induced Radiation Damage in Crystal Scintillators

    SciTech Connect

    Zhu, Ren-Yuan; Zhang, Liyuan; Yang, Fan; Ramberg, Eric; Nebel, Todd

    2014-03-11

    This is a technical scope of work (TSW) between the Fermi National Accelerator Laboratory (Fermilab) and the experimenters of California Institute of Technology who have committed to participate in beam tests to be carried out during the 2014 Fermilab Test Beam Facility program. The goal of this investigation is to understand the proton-induced radiation damage in candidate fast crystal scintillators for future HEP experiments. Degradations of the optical and scintillation properties, including emission and transmittance spectra, light output, decay time and light response uniformity, will be measured before and after each step of proton irradiation at Fermilab with a defined fluence. The irradiation will start with a fluence of 1010/cm2 and going up in four steps to 1013/cm2.

  8. Crystal growth and scintillation characterizations of Tl2LiYCl6: Ce3+

    NASA Astrophysics Data System (ADS)

    Rooh, Gul; Kim, H. J.; Park, H.; Kim, Sunghwan

    2017-02-01

    Single crystals of Tl2LiYCl6 with different mole% of Ce-concentration (0.5 and 5 mol%) were presented. This material belongs to Chloro-elpasolite crystal family and was grown by two zone vertical Bridgman technique. X-ray diffraction pattern of the Tl2LiYCl6 single crystal was measured. X-ray diffraction analysis confirmed tetragonal crystal structure. The melting point of the sample was measured by DSC. Typical Ce3+ ion emission spectra were observed when samples were excited by an X-ray source at room temperature. The observed emission spectra were located between 350 nm and 530 nm wavelength range and peaking around 430 nm. Pulse height spectra of the samples under 662 keV γ-rays excitation shows improvement in energy resolution with the increase of Ce-concentration in the host lattice. The energy resolutions were obtained to be 10.6% and 7.2% (FWHM) for 0.5% and 5% Ce3+ concentration, respectively. Under γ-ray excitation, a maximum light yield of 23,800±2400 ph/MeV was observed for 5% Ce-concentration. Studied samples of Tl2LiYCl6: Ce3+ showed three exponential decay time components under γ-ray excitation. From the measured scintillation properties, we consider this material is a promising scintillator for radiation detection.

  9. Kinetic and scintillation characteristics of CsI(Na) crystals grown under melt mixing

    NASA Astrophysics Data System (ADS)

    Goriletsky, V. I.; Grinyov, B. V.; Panova, A. M.; Shakhova, K. V.; Vinograd, E. L.; Korsunov, S. P.

    1999-10-01

    The effect of activator concentration on the γ-scintillation pulse shape, the light yield upon excitation with γ-rays and α-particles as well as the energy resolution, has been investigated for CsI(Na) crystals. The crystals were grown with a homogeneous activator distribution. Based on the concentration dependence of the α-particle light yield the number of activator emission centres in the crystals has been concluded to increase with concentration up to 2.5 × 10-2 mol% of NaI. Therefore, the maximum yield of γ-scintillation at ≈9 × 10-3 mol% NaI is due to a sufficient number of emission centres at the given ionization density. It is shown that the decay time can be reduced from 630 to 570 ns without change of the crystal spectrometric quality, and that it may be further reduced, in principle, down to values close to the decay time for intracenter excitation.

  10. Recent results and perspectives of ββ decay experiments with crystal scintillators at Gran Sasso

    SciTech Connect

    Bernabei, R.

    2013-12-30

    Crystal scintillators offer important tools to investigate ββ decay modes in various isotopes with a well known technology and the possibility of enrichment of the material in specific isotopes. Large efforts to develop and use highly radiopure dedicated detectors are carried out at Gran Sasso by the DAMA-Kiev collaboration. These efforts have allowed the investigation of many types of decay modes in several isotopes and the improvement of the existing limits or the set of new ones. A short summary on main aspects is given in this paper.

  11. Readout of undoped CsI and CeF{sub 3} crystals using scintillating fibers and bars

    SciTech Connect

    Woody, C.L.; Stoll, S.P.; Frank, J.S.

    1995-08-01

    An investigation has been made of a readout technique for undoped cesium iodide and cerium fluoride crystals using scintillating fibers and bars. The method uses the fluors in the scintillator as wavelength shifters to absorb the primary UV scintillation light from the crystals and reemit it at a longer wavelength which can be more easily propagated over large distances. A study was made for various types of fibers (BCF-10, BCF-12 and BCF-20), giving the dependence of the light output on fluor type, fiber diameter and the spacing between fibers. Similar studies are made for several types of bars (BC-404 and BC-408) which compare the light output for various bar thicknesses, flour concentrations and geometrical configurations. An initial investigation also showed that this technique can be used to read out CeF{sub 3} crystals.

  12. High speed growth of SrI2 scintillator crystals by the EFG process

    NASA Astrophysics Data System (ADS)

    Calvert, G.; Guguschev, C.; Burger, A.; Groza, M.; Derby, J. J.; Feigelson, R. S.

    2016-12-01

    Strontium iodide (SrI2), an important new scintillator crystal having a high light yield and excellent energy resolution, was grown for the first time by the edge-defined film-fed (EFG) growth method. Using high purity starting materials and floating dies made of graphite, fused quartz or AlN, large cylindrical, planar or square cross-section single crystals (12-15 mm across and >7 cm long) were produced at growth rates up to 15 mm/h, significantly faster than the current Bridgman growth technology. Details on the equipment used to grow this deliquescent material and on its growth behavior are given along with some discussion of crystalline quality.

  13. Precision machining and polishing of scintillating crystals for large calorimeters and hodoscopes

    NASA Astrophysics Data System (ADS)

    Wuest, C. R.; Fuchs, B. A.; Holdener, F. R.; Heck, J. L., Jr.

    1994-04-01

    New machining and polishing techniques have been developed for large scintillating crystal arrays such as the Barium Fluoride Electromagnetic Calorimeter for the GEM Detector at SSCL, the Crystal Clear Collaboration's cerium fluoride or lead tungstenate calorimeter at the proposed LHC and CERN, the PHENIX Detector at RHIC (barium fluoride), and the cesium iodide Calorimeter for the BaBar Detector at PEP-2 B Factory at SLAC. The machining and polishing methods to be presented in this paper provide crystalline surfaces without sub-surface damage or deformation as verified by Rutherford Back-scattering (RBS) analysis. Surface roughness of about 10-20 A and sub-micron mechanical tolerances have been demonstrated on large barium fluoride crystal samples. Mass production techniques have also been developed for machining the proper angled surfaces and polishing up to five 50 cm long crystals at one time. These techniques utilize kinematic mount technology developed at LLNL to allow precision machining and polishing of complex surfaces. They will present this technology along with detailed surface studies of barium fluoride and cerium fluoride crystals polished with this technique.

  14. Precision machining and polishing of scintillating crystals for large calorimeters and hodoscopes. Revision 1

    SciTech Connect

    Wuest, C.R.; Fuchs, B.A.; Holdener, F.R.; Heck, J.L. Jr.

    1994-04-01

    New machining and polishing techniques have been developed for large scintillating crystal arrays such as the Barium Fluoride Electromagnetic Calorimeter for the GEM Detector at SSCL, the Crystal Clear Collaboration`s cerium fluoride or lead tungstenate calorimeter at the proposed LHC and CERN, the PHENIX Detector at RHIC (barium fluoride), and the cesium iodide Calorimeter for the BaBar Detector at PEP-2 B Factory at SLAC. The machining and polishing methods to be presented in this paper provide crystalline surfaces without sub-surface damage or deformation as verified by Rutherford Back-scattering (RBS) analysis. Surface roughness of about 10--20 angstroms and sub-micron mechanical tolerances have been demonstrated on large barium fluoride crystal samples. Mass production techniques have also been developed for machining the proper angled surfaces and polishing up to five 50 cm long crystals at one time. These techniques utilize kinematic mount technology developed at LLNL to allow precision machining and polishing of complex surfaces. They will present this technology along with detailed surface studies of barium fluoride and cerium fluoride crystals polished with this technique.

  15. Research activity with different types of scintillation materials

    NASA Astrophysics Data System (ADS)

    Brinkmann, K.-T.; Borisevich, A.; Diehl, S.; Dormenev, V.; Houzvicka, J.; Korjik, M.; Novotny, R. W.; Zaunick, H.-G.; Zimmermann, S.

    2016-10-01

    Nowadays there is a growing interest and demand in the development of new types of scintillation materials for experimental high energy physics. Future detector developments will focus on cheap, fast, and radiation hard materials, especially for application in collider experiments. The most recent results obtained by the Giessen group in close cooperation with colleagues from different institutes will be presented. The new start of the mass production of high quality lead tungstate crystals (PbWO4, PWO) for electromagnetic calorimetry was started by the company CRYTUR (Turnov, Czech Republic). We will present a detailed progress report on the research program of lead tungstate performed in the last two years. The latest results in the development of LuAG:Ce, YAG:Ce and LYSO:Ce inorganic fibers, grown by the micro pulling down method and cut with the heated wire technique as well as new glass ceramics material BaO*2SiO2 (DSB) doped by Ce and Gd will be presented. In addition, different samples of the organic plastic scintillator EJ-260 produced by the company Eljen Technology (Sweetwater, USA) have been characterized. The study has focused on the change of performance after irradiation with 150 MeV protons up to an integral fluence of 5-1013 protons/cm2 as well as with a strong 60Co gamma-source accumulating an integral dose of 100 Gy.

  16. Simulation of light transport in scintillators based on 3D characterization of crystal surfaces.

    PubMed

    Roncali, Emilie; Cherry, Simon R

    2013-04-07

    In the development of positron emission tomography (PET) detectors, understanding and optimizing scintillator light collection is critical for achieving high performance, particularly when the design incorporates depth-of-interaction (DOI) encoding or time-of-flight information. Monte-Carlo simulations play an important role in guiding research in detector designs and popular software such as GATE now include models of light transport in scintillators. Although current simulation toolkits are able to provide accurate models of perfectly polished surfaces, they do not successfully predict light output for other surface finishes, for example those often used in DOI-encoding detectors. The lack of accuracy of those models mainly originates from a simplified description of rough surfaces as an ensemble of micro-facets determined by the distribution of their normal, typically a gaussian distribution. The user can specify the standard deviation of this distribution, but this parameter does not provide a full description of the surface reflectance properties. We propose a different approach based on 3D measurements of the surface using atomic force microscopy. Polished and rough (unpolished) crystals were scanned to compute the surface reflectance properties. The angular distributions of reflectance and reflected rays were computed and stored in look-up tables (LUTs). The LUTs account for the effect of incidence angle and were integrated in a light transport model. Crystals of different sizes were simulated with and without reflector. The simulated maximum light output and the light output as a function of DOI showed very good agreement with experimental characterization of the crystals, indicating that our approach provides an accurate model of polished and rough surfaces and could be used to predict light collection in scintillators. This model is based on a true 3D representation of the surface, makes no assumption about the surface and provides insight on the optical

  17. Simulation of light transport in scintillators based on 3D characterization of crystal surfaces

    NASA Astrophysics Data System (ADS)

    Roncali, Emilie; Cherry, Simon R.

    2013-04-01

    In the development of positron emission tomography (PET) detectors, understanding and optimizing scintillator light collection is critical for achieving high performance, particularly when the design incorporates depth-of-interaction (DOI) encoding or time-of-flight information. Monte-Carlo simulations play an important role in guiding research in detector designs and popular software such as GATE now include models of light transport in scintillators. Although current simulation toolkits are able to provide accurate models of perfectly polished surfaces, they do not successfully predict light output for other surface finishes, for example those often used in DOI-encoding detectors. The lack of accuracy of those models mainly originates from a simplified description of rough surfaces as an ensemble of micro-facets determined by the distribution of their normal, typically a Gaussian distribution. The user can specify the standard deviation of this distribution, but this parameter does not provide a full description of the surface reflectance properties. We propose a different approach based on 3D measurements of the surface using atomic force microscopy. Polished and rough (unpolished) crystals were scanned to compute the surface reflectance properties. The angular distributions of reflectance and reflected rays were computed and stored in look-up tables (LUTs). The LUTs account for the effect of incidence angle and were integrated in a light transport model. Crystals of different sizes were simulated with and without reflector. The simulated maximum light output and the light output as a function of DOI showed very good agreement with experimental characterization of the crystals, indicating that our approach provides an accurate model of polished and rough surfaces and could be used to predict light collection in scintillators. This model is based on a true 3D representation of the surface, makes no assumption about the surface and provides insight on the optical

  18. Luminescence and scintillation properties of Tl- and Ce-doped Cs2HfCl6 crystals

    NASA Astrophysics Data System (ADS)

    Saeki, Keiichiro; Fujimoto, Yutaka; Koshimizu, Masanori; Nakauchi, Daisuke; Tanaka, Hironori; Yanagida, Takayuki; Asai, Keisuke

    2017-02-01

    The luminescence and scintillation properties of Tl- and Ce-doped Cs2HfCl6 crystals were investigated by photoluminescence and radioluminescence spectroscopy. In the photoluminescence spectra, emission bands of the activators were observed at 500 nm for Tl-doped Cs2HfCl6, and at 340 and 380 nm for Ce-doped Cs2HfCl6. The radioluminescence bands were observed at 405 and 430 nm for Tl- and Ce-doped Cs2HfCl6, respectively. Scintillation decay time constants for the Tl- and Ce-doped Cs2HfCl6 were smaller than those for the corresponding undoped crystals. Scintillation light yields for Tl- and Ce-doped Cs2HfCl6 were estimated to be 23,700 and 15,700 photons/MeV, respectively.

  19. In situ diagnostics of the crystal-growth process through neutron imaging: application to scintillators

    PubMed Central

    Tremsin, Anton S.; Makowska, Małgorzata G.; Perrodin, Didier; Shalapska, Tetiana; Khodyuk, Ivan V.; Trtik, Pavel; Boillat, Pierre; Vogel, Sven C.; Losko, Adrian S.; Strobl, Markus; Kuhn, L. Theil; Bizarri, Gregory A.; Bourret-Courchesne, Edith D.

    2016-01-01

    Neutrons are known to be unique probes in situations where other types of radiation fail to penetrate samples and their surrounding structures. In this paper it is demonstrated how thermal and cold neutron radiography can provide time-resolved imaging of materials while they are being processed (e.g. while growing single crystals). The processing equipment, in this case furnaces, and the scintillator materials are opaque to conventional X-ray interrogation techniques. The distribution of the europium activator within a BaBrCl:Eu scintillator (0.1 and 0.5% nominal doping concentrations per mole) is studied in situ during the melting and solidification processes with a temporal resolution of 5–7 s. The strong tendency of the Eu dopant to segregate during the solidification process is observed in repeated cycles, with Eu forming clusters on multiple length scales (only for clusters larger than ∼50 µm, as limited by the resolution of the present experiments). It is also demonstrated that the dopant concentration can be quantified even for very low concentration levels (∼0.1%) in 10 mm thick samples. The interface between the solid and liquid phases can also be imaged, provided there is a sufficient change in concentration of one of the elements with a sufficient neutron attenuation cross section. Tomographic imaging of the BaBrCl:0.1%Eu sample reveals a strong correlation between crystal fractures and Eu-deficient clusters. The results of these experiments demonstrate the unique capabilities of neutron imaging for in situ diagnostics and the optimization of crystal-growth procedures. PMID:27275133

  20. Exploring growth conditions and Eu2+ concentration effects for KSr2I5:Eu scintillator crystals

    NASA Astrophysics Data System (ADS)

    Stand, L.; Zhuravleva, M.; Camarda, G.; Lindsey, A.; Johnson, J.; Hobbs, C.; Melcher, C. L.

    2016-04-01

    Our current research is focused on understanding dopant optimization, growth rate, homogeneity and their impact on the overall performance of KSr2I5:Eu2+ single crystal scintillators. In this work we have investigated the effects of Eu2+ concentration in the potassium strontium iodide matrix, and we found that the concentration needed to maximize the light yield was 4 mol%. In order to assess the effects of the pulling rate, we grew single crystals at 12, 24 and 120 mm/day via the vertical Bridgman technique. For the sample sizes measured (5×5×5 mm3), we found that the crystal grown at the fastest rate of 120 mm/day showed a light yield within ~7% of the more slowly grown boules, and no significant change was observed in the energy resolution. Therefore, light yields from 88,000 to 96,000 ph/MeV and energy resolutions from 2.4 to 3.0% (at 662 keV) were measured for KSr2I5:Eu 4% over a relatively wide range of growth conditions. In order to assess the homogeneity of KSr2I5:Eu 4%, a newly developed micro-resolution X-ray technique was used to map the light yield as a function of excitation position. In the crystals that we studied, we did not observe any significant inhomogeneity other than a smooth gradient due to light collection and self absorption effects.

  1. SiPM optical crosstalk amplification due to scintillator crystal: effects on timing performance.

    PubMed

    Gola, Alberto; Ferri, Alessandro; Tarolli, Alessandro; Zorzi, Nicola; Piemonte, Claudio

    2014-07-07

    For a given photon detection efficiency (PDE), the primary, Poisson distributed, dark count rate of the detector (DCR0) is one of the most limiting factors affecting the timing resolution of a silicon photomultiplier (SiPM) in the scintillation light readout. If the effects of DCR0 are removed through a suitable baseline compensation algorithm or by cooling, it is possible to clearly observe another phenomenon that limits the PDE, and thus the timing resolution of the detector. It is caused by the optical crosstalk of the SiPM, which is significantly increased by the presence of the scintillator. In this paper, we describe this phenomenon, which is also easily observed from the reverse I-V curve of the device, and we relate it to the measured coincidence resolving time in 511 keV γ-ray measurements. We discuss its consequences on the SiPM design and, in particular, we observe that there is an optimal cell size, dependent on both SiPM and crystal parameters, that maximizes the PDE in presence of optical crosstalk. Finally, we report on a crosstalk simulator developed to study the phenomenon and we compare the simulation results obtained for different SiPM technologies, featuring different approaches to the reduction of the crosstalk.

  2. Defect Engineering in SrI2:Eu2+ Single Crystal Scintillators

    SciTech Connect

    Wu, Yuntao; Boatner, Lynn A.; Lindsey, Adam C.; Zhuravleva, Mariya; Jones, Steven; Auxier, John D.; Hall, Howard L.; Melcher, Charles L.

    2015-06-23

    Eu2+-activated strontium iodide is an excellent single crystal scintillator used for gamma-ray detection and significant effort is currently focused on the development of large-scale crystal growth techniques. A new approach of molten-salt pumping or so-called melt aging was recently applied to optimize the crystal quality and scintillation performance. Nevertheless, a detailed understanding of the underlying mechanism of this technique is still lacking. The main purpose of this paper is to conduct an in-depth study of the interplay between microstructure, trap centers and scintillation efficiency after melt aging treatment. Three SrI2:2 mol% Eu2+ single crystals with 16 mm diameter were grown using the Bridgman method under identical growth conditions with the exception of the melt aging time (e.g. 0, 24 and 72 hours). Using energy-dispersive X-ray spectroscopy, it is found that the matrix composition of the finished crystal after melt aging treatment approaches the stoichiometric composition. The mechanism responsible for the formation of secondary phase inclusions in melt-aged SrI2:Eu2+ is discussed. Simultaneous improvement in light yield, energy resolution, scintillation decay-time and afterglow is achieved in melt-aged SrI2:Eu2+. The correlation between performance improvement and defect structure is addressed. The results of this paper lead to a better understanding of the effects of defect engineering in control and optimization of metal halide scintillators using the melt aging technique.

  3. New Tl2LaBr5: Ce3+ crystal scintillator for γ-rays detection

    NASA Astrophysics Data System (ADS)

    Kim, H. J.; Rooh, Gul; Khan, Arshad; Kim, Sunghwan

    2017-03-01

    In this study we present our preliminary report on the scintillation properties of new Ce-doped Tl2LaBr5 single crystal. Two zones vertical Bridgman technique is used for the growth of this compound. Pure and Ce-doped samples showed maximum emission peaks at 435 nm and 415 nm, respectively. Best light yield of 43,000±4300 ph/MeV with 6.3% (FWHM) energy resolution is obtained for 5% Ce-doped sample under γ-ray excitation. Single exponential decay time constant of 25 ns is observed for 5% Ce doped sample. Effective Z-number is found to be 67, therefore efficient detection of X- and γ-ray will be possible. Preliminary results revealed that this compound will be an ideal candidate for the medical imaging techniques. Further investigations are under way for the determination of optimized conditions of this compound.

  4. Enhancement of directional broadband luminescence from a scintillation film via guided-mode resonance in a photonic crystal structure

    NASA Astrophysics Data System (ADS)

    Zhu, Zhichao; Liu, Bo; Cheng, Chuanwei; Zhang, Haifeng; Chen, Hong; Gu, Mu; Liu, Jinliang; Chen, Liang; Ouyang, Xiaoping; Xue, Chaofan; Wu, Yanqing

    2017-01-01

    Scintillation films play an important role in radiation detection. Improved light output and control of emission directionality are critical for practical applications. To obtain enhancement of broadband directional luminescence from a Lu2SiO5:Ce3+ scintillation film, a special photonic crystal structure is deposited on the film surface to provide multiple guided-mode resonances. The structure can be designed according to the application requirements. Numerical simulations are performed to analyze the enhancement. Overall, this method could be used when directional emission is required for radiation detection.

  5. Enhanced light extraction of scintillator using large-area photonic crystal structures fabricated by soft-X-ray interference lithography

    SciTech Connect

    Zhu, Zhichao; Wu, Shuang; Liu, Bo Cheng, Chuanwei; Gu, Mu; Chen, Hong; Xue, Chaofan; Zhao, Jun; Wang, Liansheng; Wu, Yanqing; Tai, Renzhong

    2015-06-15

    Soft-X-ray interference lithography is utilized in combination with atomic layer deposition to prepare photonic crystal structures on the surface of Bi{sub 4}Ge{sub 3}O{sub 12} (BGO) scintillator in order to extract the light otherwise trapped in the internal of scintillator due to total internal reflection. An enhancement with wavelength- and emergence angle-integration by 95.1% has been achieved. This method is advantageous to fabricate photonic crystal structures with large-area and high-index-contrast which enable a high-efficient coupling of evanescent field and the photonic crystal structures. Generally, the method demonstrated in this work is also suitable for many other light emitting devices where a large-area is required in the practical applications.

  6. Comparative analysis of the scintillation and thermoluminescent properties of Ce-doped LSO and YSO crystals and films

    NASA Astrophysics Data System (ADS)

    Zorenko, Yu.; Gorbenko, V.; Bilski, P.; Twardak, A.; Mandowska, E.; Mandowski, A.; Sidletskiy, O.

    2014-08-01

    The work is devoted to the comparative analysis of the scintillation and thermoluminescent properties of the undoped and Ce-doped A2SiO5 (A = Lu, Y) orthosilicates, prepared in single crystal form by the Czochralski method and in the form of single crystalline film using the liquid phase epitaxy method. We have found that differences in the methods of material preparation resulted in the significant differences in the scintillation and thermoluminescent properties of undoped and Ce doped YSO and LSO crystals and films. Such differences are caused by the presence or absence of main host defects (first of all, oxygen vacancies and flux related impurities) as emission and trapping centers in YSO and LSO crystals and films.

  7. Characterization of Pr:LuAG scintillating crystals for X-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Bertoni, R.; Bonesini, M.; Cervi, T.; Clemenza, M.; De Bari, A.; Falcone, A.; Mazza, R.; Menegolli, A.; Nastasi, M.; Rossella, M.

    2016-07-01

    The main features of the Pr doped Lu3Al5O12 (Pr:LuAG) scintillating crystals for X-ray spectroscopy applications have been studied using different radioactive sources and photo-detectors. Pr:LuAG is cheaper, compared to a Germanium detector, but with remarkable properties which make it useful for many applications, from fundamental physics measurements to the PET imaging for medical purposes: high density, elevate light yield, fast response, high energy resolution, no hygroscopicity. A sample of Pr:LuAG crystals with 14 mm×14 mm surface area and 13 mm thickness and a NaI crystal of the same surface and 26 mm thickness used as a reference have been characterized with several radioactive sources, emitting photons in the range 100-1000keV. Different light detectors were adopted for the Pr:LuAG studies, sensitive to its UV emission (peak at 310 nm): a 3 in. PMT (Hamamatsu R11065) and new arrays of Hamamatsu SiPM S13361, with siliconic resin as a window. Preliminary results are presented on the performance of the Pr:LuAG crystals, to be mounted in a 2 × 2 array to be tested in the 2015 run of the FAMU experiment at RIKEN-RAL muon facility. The goal is the detection of the X-rays (around 130 keV) emitted during the de-excitation processes of the muonic hydrogen after the excitation with an IR laser with wavelength set at the resonance of the hyperfine splitting, to measure the muonic atom proton radius with unprecedented precision.

  8. Crystal growth and characterization of rare earth iodides for scintillation detection

    NASA Astrophysics Data System (ADS)

    van Loef, E. V.; Higgins, W. M.; Glodo, J.; Churilov, A. V.; Shah, K. S.

    2008-04-01

    In this paper we report on the crystal growth and characterization of a new class of inorganic scintillators based on the rare earth iodides, in particular LuI 3, YI 3 and GdI 3, doped with trivalent cerium. Single crystals of LuI 3:Ce 3+, YI 3:Ce 3+ and GdI 3:Ce 3+ were grown by the vertical Bridgman technique in evacuated silica ampoules. In some cases, tantalum or graphite crucibles were used to minimize wetting of the ampoule. X-ray excited optical luminescence spectra of LuI 3:Ce 3+, YI 3:Ce 3+ and GdI 3:Ce 3+ exhibit a broad band due to Ce 3+ emission, peaking in the 500-550 nm region. LuI 3:Ce 3+, YI 3:Ce 3+ and GdI 3:Ce 3+ show high light yields up to 100,000 photons/MeV and fast principle decay time constants of <40 ns. Energy resolutions measured at 662 keV are of the order of 3.5-9% (FWHM).

  9. Analytical calculation of the lower bound on timing resolution for PET scintillation detectors comprising high-aspect-ratio crystal elements

    NASA Astrophysics Data System (ADS)

    Cates, Joshua W.; Vinke, Ruud; Levin, Craig S.

    2015-07-01

    Excellent timing resolution is required to enhance the signal-to-noise ratio (SNR) gain available from the incorporation of time-of-flight (ToF) information in image reconstruction for positron emission tomography (PET). As the detector’s timing resolution improves, so does SNR, reconstructed image quality, and accuracy. This directly impacts the challenging detection and quantification tasks in the clinic. The recognition of these benefits has spurred efforts within the molecular imaging community to determine to what extent the timing resolution of scintillation detectors can be improved and develop near-term solutions for advancing ToF-PET. Presented in this work, is a method for calculating the Cramér-Rao lower bound (CRLB) on timing resolution for scintillation detectors with long crystal elements, where the influence of the variation in optical path length of scintillation light on achievable timing resolution is non-negligible. The presented formalism incorporates an accurate, analytical probability density function (PDF) of optical transit time within the crystal to obtain a purely mathematical expression of the CRLB with high-aspect-ratio (HAR) scintillation detectors. This approach enables the statistical limit on timing resolution performance to be analytically expressed for clinically-relevant PET scintillation detectors without requiring Monte Carlo simulation-generated photon transport time distributions. The analytically calculated optical transport PDF was compared with detailed light transport simulations, and excellent agreement was found between the two. The coincidence timing resolution (CTR) between two 3× 3× 20 mm3 LYSO:Ce crystals coupled to analogue SiPMs was experimentally measured to be 162+/- 1 ps FWHM, approaching the analytically calculated lower bound within 6.5%.

  10. Analytical Calculation of the Lower Bound on Timing Resolution for PET Scintillation Detectors Comprising High-Aspect-Ratio Crystal Elements

    PubMed Central

    Cates, Joshua W.; Vinke, Ruud; Levin, Craig S.

    2015-01-01

    Excellent timing resolution is required to enhance the signal-to-noise ratio (SNR) gain available from the incorporation of time-of-flight (ToF) information in image reconstruction for positron emission tomography (PET). As the detector’s timing resolution improves, so does SNR, reconstructed image quality, and accuracy. This directly impacts the challenging detection and quantification tasks in the clinic. The recognition of these benefits has spurred efforts within the molecular imaging community to determine to what extent the timing resolution of scintillation detectors can be improved and develop near-term solutions for advancing ToF-PET. Presented in this work, is a method for calculating the Cramér-Rao lower bound (CRLB) on timing resolution for scintillation detectors with long crystal elements, where the influence of the variation in optical path length of scintillation light on achievable timing resolution is non-negligible. The presented formalism incorporates an accurate, analytical probability density function (PDF) of optical transit time within the crystal to obtain a purely mathematical expression of the CRLB with high-aspect-ratio (HAR) scintillation detectors. This approach enables the statistical limit on timing resolution performance to be analytically expressed for clinically-relevant PET scintillation detectors without requiring Monte Carlo simulation-generated photon transport time distributions. The analytically calculated optical transport PDF was compared with detailed light transport simulations, and excellent agreement was found between the two. The coincidence timing resolution (CTR) between two 3×3×20 mm3 LYSO:Ce crystals coupled to analogue SiPMs was experimentally measured to be 162±1 ps FWHM, approaching the analytically calculated lower bound within 6.5%. PMID:26083559

  11. Optimizing light transport in scintillation crystals for time-of-flight PET: an experimental and optical Monte Carlo simulation study.

    PubMed

    Berg, Eric; Roncali, Emilie; Cherry, Simon R

    2015-06-01

    Achieving excellent timing resolution in gamma ray detectors is crucial in several applications such as medical imaging with time-of-flight positron emission tomography (TOF-PET). Although many factors impact the overall system timing resolution, the statistical nature of scintillation light, including photon production and transport in the crystal to the photodetector, is typically the limiting factor for modern scintillation detectors. In this study, we investigated the impact of surface treatment, in particular, roughening select areas of otherwise polished crystals, on light transport and timing resolution. A custom Monte Carlo photon tracking tool was used to gain insight into changes in light collection and timing resolution that were observed experimentally: select roughening configurations increased the light collection up to 25% and improved timing resolution by 15% compared to crystals with all polished surfaces. Simulations showed that partial surface roughening caused a greater number of photons to be reflected towards the photodetector and increased the initial rate of photoelectron production. This study provides a simple method to improve timing resolution and light collection in scintillator-based gamma ray detectors, a topic of high importance in the field of TOF-PET. Additionally, we demonstrated utility of our Monte Carlo simulation tool to accurately predict the effect of altering crystal surfaces on light collection and timing resolution.

  12. Excellent pulse height uniformity response of a new LaBr3:Ce scintillation crystal for gamma ray imaging

    NASA Astrophysics Data System (ADS)

    Pani, R.; Cinti, M. N.; Fabbri, A.; Orlandi, C.; Pellegrini, R.; Scafè, R.; Colarieti-Tosti, M.

    2015-07-01

    Nuclear Medicine SPECT imaging is taking on new challenges, regarding the improvement of quality and contrast of images. In order to reach this goal, energy resolution and Compton rejection capability have to be enhanced. For detectors based on scintillation crystal, the choice of a scintillator with high light yield is suitable; recently one of the major candidates is Lanthanum Tri-Bromide (LaBr3:Ce), with its high 63,000 ph/MeV light yield. Unfortunately, LaBr3:Ce suffers size limitations due to the actual growth techniques (maximum 3 in. diameter) and has also elevated cost. For these reasons, great interest is shown on small field of view detectors based on LaBr3:Ce, thought for imaging of specific physiological process or organ. To improve energy resolution, continuous crystals are more appropriate instead than pixelated ones. Since in a continuous crystal a decrease in position linearity, due to the light reflections, is typically obtained at the edges, an absorbent treatment of surfaces is generally utilized for SPECT applications. On the other hand, light absorption causes a relevant degradation of local energy resolution and pulse height uniformity response, affecting local image contrast. In this work an analysis on a new continuous LaBr3:Ce scintillation crystal with size proper to a small field of view gamma imager but with reflective treatment of surfaces is presented. This leads up to outstanding overall and local energy resolution results and excellent pulse height uniformity response on the whole field of view. Furthermore, preliminary imaging results are satisfactory, compared to the ones from a scintillation crystal with absorbent edges.

  13. Scintillator materials for calorimetry

    SciTech Connect

    Weber, M.J.

    1994-09-01

    Requirements for fast, dense scintillator materials for calorimetry in high energy physics and approaches to satisfying these requirements are reviewed with respect to possible hosts and luminescent species. Special attention is given to cerium-activated crystals, core-valence luminescence, and glass scintillators. The present state of the art, limitations, and suggestions for possible new scintillator materials are presented.

  14. Monte Carlo and Lambertian light guide models of the light output from scintillation crystals at megavoltage energies

    SciTech Connect

    Evans, Philip M.; Mosleh-Shirazi, M. Amin; Harris, Emma J.; Seco, Joao

    2006-06-15

    A new model of the light output from single-crystal scintillators in megavoltage energy x-ray beams has been developed, based on the concept of a Lambertian light guide model (LLG). This was evaluated in comparison with a Monte Carlo (MC) model of optical photon transport, previously developed and reported in the literature, which was used as a gold standard. The LLG model was developed to enable optimization of scintillator detector design. In both models the dose deposition and light propagation were decoupled, the scintillators were cuboids, split into a series of cells as a function of depth, with Lambertian side and entrance faces, and a specular exit face. The signal in a sensor placed 1 and 1000 mm beyond the exit face was calculated. Cesium iodide (CSI) crystals of 1.5 and 3 mm square cross section and 1, 5, and 10 mm depth were modeled. Both models were also used to determine detector signal and optical gain factor as a function of CsI scintillator thickness, from 2 to 10 mm. Results showed a variation in light output with position of dose deposition of a factor of up to approximately 5, for long, thin scintillators (such as 10x1.5x1.5 mm{sup 3}). For short, fat scintillators (such as 1x3x3 mm{sup 3}) the light output was more uniform with depth. MC and LLG generally agreed to within 5%. Results for a sensor distance of 1 mm showed an increase in light output the closer the light originates to the exit face, while a distance of 1000 mm showed a decrease in light output the closer the light originates to the exit face. For a sensor distance of 1 mm, the ratio of signal for a 10 mm scintillator to that for a 2 mm scintillator was 1.98, whereas for the 1000 mm distance the ratio was 3.00. The ratio of quantum efficiency (QE) between 10 and 2 mm thicknesses was 4.62. We conclude that these models may be used for detector optimization, with the light guide model suitable for parametric study.

  15. Imaging characterization of a new gamma ray detector based on CRY019 scintillation crystal for PET and SPECT applications

    NASA Astrophysics Data System (ADS)

    Polito, C.; Pani, R.; Trigila, C.; Cinti, M. N.; Fabbri, A.; Frantellizzi, V.; De Vincentis, G.; Pellegrini, R.; Pani, R.

    2017-02-01

    In the last 40 years, in the field of Molecular Medicine imaging there has been a huge growth in the employment and in the improvement of detectors for PET and SPECT applications in order to reach accurate diagnosis of the diseases. The most important feature required to these detectors is an high quality of images that is usually obtained benefitting from the development of a wide number of new scintillation crystals with high imaging performances. In this contest, features like high detection efficiency, short decay time, great spectral match with photodetectors, absence of afterglow and low costs are surely attractive. However, there are other factors playing an important role in the realization of high quality images such as energy and spatial resolutions, position linearity and contrast resolution. With the aim to realize an high performace gamma ray detector for PET and SPECT applications, this work is focused on the evaluation of the imaging characteristics of a recently developed scintillation crystal, CRY019.

  16. Stimulated recovery of the optical transmission of PbWO 4 scintillation crystals for electromagnetic calorimeters after radiation damage

    NASA Astrophysics Data System (ADS)

    Dormenev, V.; Kuske, T.; Novotny, R. W.; Borisevich, A.; Fedorov, A.; Korjik, M.; Mechinski, V.; Missevitch, O.; Lugert, S.

    2010-11-01

    In this paper we describe the phenomenon of the stimulated recovery of radiation damage in lead tungstate scintillation crystals achieved via illumination by visible and infrared light. It allows fast and efficient in-situ recovery of the optical transmission either during beam-off periods or on-line during data accumulation. The application can substantially improve or extend the running period of the experiment by keeping the damage at a tolerable level.

  17. Growth of shape-controlled Ce:Y3Al5O12 scintillator crystal and their scintillation properties

    NASA Astrophysics Data System (ADS)

    Yokota, Yuui; Kurosawa, Shunsuke; Ohasi, Yuji; Kamada, Kei; Yoshikawa, Akira

    2016-10-01

    A shape-controlled Ce doped Y3Al5O12 (Ce:YAG) single crystal has been grown by a micro-pulling-down method using an Ir crucible with a square die. The as-grown Ce:YAG single crystal has square-shape and flat surfaces with high transparency. The shape-controlled Ce:YAG single crystal showed more than 70% transmittance from 530 nm to 900 nm without any cutting and polishing. An emission peak around 540 nm was observed in the radioluminescence spectrum under X-ray irradiation. In addition, the light yield and energy resolution under γ-ray irradiation of the as-grown crystal without any cutting and polishing were approximately 23,000 pH/MeV and 16%, respectively.

  18. Growth and scintillation characterization of Ce3+-doped Rb2LiGdBr6 single crystals

    NASA Astrophysics Data System (ADS)

    Rooh, Gul; Kim, H. J.; Kim, Sunghwan; Khan, Sajid

    2016-10-01

    Growth and scintillation characterizations of the newly developed cerium doped Rb2LiGdBr6 (RLGB) single crystals were investigated. RLGB, which belongs to bromo-elpasolite crystal family, was grown by the vertical Bridgman technique with nominally 1%, 5%, and 10% Ce3+-concentration (mole%). X-ray excited luminescence spectra show typical Ce3+ bands between 350 to 460 nm wavelength regions. A good energy resolution of 5.5% (FWHM) and light yield of 25,500±2600 ph/MeV for 662 keV γ-rays were observed at 5% Ce3+-concentration. Under γ-ray excitation, RLGB:Ce3+ crystals display multi-exponential decays with Ce3+ like decay components at 23 ns and 29 ns for 1% and 5% Ce-concentrations, respectively. From the results, it is expected that this scintillator could be used as a thermal neutron detector because of Li and Gd ions in the host lattice. Also, like other inorganic halide scintillators, it is very hygroscopic.

  19. Characterization of scintillator crystals for usage as prompt gamma monitors in particle therapy

    NASA Astrophysics Data System (ADS)

    Roemer, K.; Pausch, G.; Bemmerer, D.; Berthel, M.; Dreyer, A.; Golnik, C.; Hueso-González, F.; Kormoll, T.; Petzoldt, J.; Rohling, H.; Thirolf, P.; Wagner, A.; Wagner, L.; Weinberger, D.; Fiedler, F.

    2015-10-01

    Particle therapy in oncology is advantageous compared to classical radiotherapy due to its well-defined penetration depth. In the so-called Bragg peak, the highest dose is deposited; the tissue behind the cancerous area is not exposed. Different factors influence the range of the particle and thus the target area, e.g. organ motion, mispositioning of the patient or anatomical changes. In order to avoid over-exposure of healthy tissue and under-dosage of cancerous regions, the penetration depth of the particle has to be monitored, preferably already during the ongoing therapy session. The verification of the ion range can be performed using prompt gamma emissions, which are produced by interactions between projectile and tissue, and originate from the same location and time of the nuclear reaction. The prompt gamma emission profile and the clinically relevant penetration depth are correlated. Various imaging concepts based on the detection of prompt gamma rays are currently discussed: collimated systems with counting detectors, Compton cameras with (at least) two detector planes, or the prompt gamma timing method, utilizing the particle time-of-flight within the body. For each concept, the detection system must meet special requirements regarding energy, time, and spatial resolution. Nonetheless, the prerequisites remain the same: the gamma energy region (2 to 10 MeV), high counting rates and the stability in strong background radiation fields. The aim of this work is the comparison of different scintillation crystals regarding energy and time resolution for optimized prompt gamma detection.

  20. Metal-organic scintillator crystals for X-ray, gamma ray, and neutron detection

    DOEpatents

    Boatner, Lynn A [Oak Ridge, TN; Kolopus, James A [Clinton, TN; Neal, John S [Knoxville, TN; Ramey, Joanne Oxendine [Knoxville, TN; Wisniewski, Dariusz J [Torun, PL

    2012-01-03

    New metal-organic materials are useful as scintillators and have the chemical formula LX.sub.3(CH.sub.3OH).sub.4 where L is Y, Sc, or a lanthanide element, and X is a halogen element. An example of the scintillator materials is CeCl.sub.3(CH.sub.3OH).sub.4.

  1. Side readout of long scintillation crystal elements with digital SiPM for TOF-DOI PET

    SciTech Connect

    Yeom, Jung Yeol E-mail: cslevin@stanford.edu; Vinke, Ruud; Levin, Craig S. E-mail: cslevin@stanford.edu

    2014-12-15

    Purpose: Side readout of scintillation light from crystal elements in positron emission tomography (PET) is an alternative to conventional end-readout configurations, with the benefit of being able to provide accurate depth-of-interaction (DOI) information and good energy resolution while achieving excellent timing resolution required for time-of-flight PET. This paper explores different readout geometries of scintillation crystal elements with the goal of achieving a detector that simultaneously achieves excellent timing resolution, energy resolution, spatial resolution, and photon sensitivity. Methods: The performance of discrete LYSO scintillation elements of different lengths read out from the end/side with digital silicon photomultipliers (dSiPMs) has been assessed. Results: Compared to 3 × 3 × 20 mm{sup 3} LYSO crystals read out from their ends with a coincidence resolving time (CRT) of 162 ± 6 ps FWHM and saturated energy spectra, a side-readout configuration achieved an excellent CRT of 144 ± 2 ps FWHM after correcting for timing skews within the dSiPM and an energy resolution of 11.8% ± 0.2% without requiring energy saturation correction. Using a maximum likelihood estimation method on individual dSiPM pixel response that corresponds to different 511 keV photon interaction positions, the DOI resolution of this 3 × 3 × 20 mm{sup 3} crystal side-readout configuration was computed to be 0.8 mm FWHM with negligible artifacts at the crystal ends. On the other hand, with smaller 3 × 3 × 5 mm{sup 3} LYSO crystals that can also be tiled/stacked to provide DOI information, a timing resolution of 134 ± 6 ps was attained but produced highly saturated energy spectra. Conclusions: The energy, timing, and DOI resolution information extracted from the side of long scintillation crystal elements coupled to dSiPM have been acquired for the first time. The authors conclude in this proof of concept study that such detector configuration has the potential to enable

  2. Side readout of long scintillation crystal elements with digital SiPM for TOF-DOI PET

    PubMed Central

    Yeom, Jung Yeol; Vinke, Ruud; Levin, Craig S.

    2014-01-01

    Purpose: Side readout of scintillation light from crystal elements in positron emission tomography (PET) is an alternative to conventional end-readout configurations, with the benefit of being able to provide accurate depth-of-interaction (DOI) information and good energy resolution while achieving excellent timing resolution required for time-of-flight PET. This paper explores different readout geometries of scintillation crystal elements with the goal of achieving a detector that simultaneously achieves excellent timing resolution, energy resolution, spatial resolution, and photon sensitivity. Methods: The performance of discrete LYSO scintillation elements of different lengths read out from the end/side with digital silicon photomultipliers (dSiPMs) has been assessed. Results: Compared to 3 × 3 × 20 mm3 LYSO crystals read out from their ends with a coincidence resolving time (CRT) of 162 ± 6 ps FWHM and saturated energy spectra, a side-readout configuration achieved an excellent CRT of 144 ± 2 ps FWHM after correcting for timing skews within the dSiPM and an energy resolution of 11.8% ± 0.2% without requiring energy saturation correction. Using a maximum likelihood estimation method on individual dSiPM pixel response that corresponds to different 511 keV photon interaction positions, the DOI resolution of this 3 × 3 × 20 mm3 crystal side-readout configuration was computed to be 0.8 mm FWHM with negligible artifacts at the crystal ends. On the other hand, with smaller 3 × 3 × 5 mm3 LYSO crystals that can also be tiled/stacked to provide DOI information, a timing resolution of 134 ± 6 ps was attained but produced highly saturated energy spectra. Conclusions: The energy, timing, and DOI resolution information extracted from the side of long scintillation crystal elements coupled to dSiPM have been acquired for the first time. The authors conclude in this proof of concept study that such detector configuration has the potential to enable outstanding

  3. X-ray Luminescence Efficiency of GAGG:Ce Single Crystal Scintillators for use in Tomographic Medical Imaging Systems

    NASA Astrophysics Data System (ADS)

    David, S. L.; Valais, I. G.; Michail, C. M.; Kandarakis, I. S.

    2015-09-01

    The purpose of the present study was to evaluate different scintillator crystal samples, with a cross section of 3×3mm2 and various thicknesses ranging from 4mm up to 20mm, of the new mixed Gd3Al2Ga3O12:Ce (GAGG:Ce) scintillator material under X-ray irradiation, for potential applications in Tomographic Medical Imaging systems. Evaluation was performed by determining the X-ray luminescence efficiency (XLE) (emitted light energy flux over incident X-ray energy flux) in energies employed in general X-ray imaging. For the luminescence efficiency measurements, the scintillator samples were exposed to X-rays using a BMI General Medical Merate tube, with rotating Tungsten anode and inherent filtration equivalent to 2 mm Al. X-ray tube voltages between 50 to 130 kV were selected. An additional 20 mm filtration was introduced to the beam to simulate beam quality alternation equivalent to a human body. The emitted light energy flux measurements were performed using an experimental set up comprising a light integration sphere coupled to an EMI 9798B photomultiplier tube which was connected to a Cary 401 vibrating reed electrometer. The GAGG:Ce sample with dimensions 3×3×10 mm3 exhibited higher XLE values, in the whole X- ray energy range examined. XLE value equal to 0.013 was recorded for this crystal at 130 kVp - a setting frequently used in Computed Tomography applications.

  4. Luminescent and scintillation properties of Lu3Al5O12:Sc single crystal and single crystalline films

    NASA Astrophysics Data System (ADS)

    Zorenko, Y.; Gorbenko, V.; Voznyak, T.; Savchyn, V.; Nizhankovskiy, S.; Dan'ko, A.; Puzikov, V.; Laguta, V.; Mares, J. A.; Nikl, M.; Nejezchleb, K.; Batentschuk, M.; Winnacker, A.

    2012-10-01

    The work is dedicated to growth by the liquid phase epitaxy method and study of the luminescence and scintillation properties of Sc3+ doped single crystalline films (SCF) of Lu3Al5O12 (LuAG) garnet. The scintillation properties of SCF are compared with single crystal (SC) analogues grown by the Horizontal Direct Crystallization and Czochralski methods. We consider the dependence of intensity of the Sc3+ emission in LuAG host on the activator concentration and influence of flux contamination on the light yield (LY) of the Sc3+ luminescence in LuAG:Sc SCF with respect to their SC counterparts and the reference YAP:Ce scintillator. From the NMR investigations of LuAG:Sc SCF we confirm the substitution by Sc3+ ions both the octahedral and dodecahedral positions of LuAG host and formation of the ScAl and ScLu related emission centers, respectively. We also show that the luminescence spectrum in the UV range and decay kinetics of LuAG:Sc SCF can be effectively tuned by changing the scandium content.

  5. Polishing procedure and surface characterization lead tungstate crystal scintillator Road No. 723 and No. 754

    SciTech Connect

    Kellam, M

    1996-05-01

    Step by step procedures are given for polishing the scintillator rods. A Strasbaugh spindle polishing machine was used along with visual inspection and hand polishing. Extensive data is given on pre-polish surface characterization, profilometry, microphotography, and interferometry.

  6. Effects of Mg-codoping on luminescence and scintillation properties of Ce doped Lu3(Ga,Al)5O12 single crystals

    NASA Astrophysics Data System (ADS)

    Yamaguchi, Hiroaki; Kamada, Kei; Pejchal, Jan; Kurosawa, Shunsuke; Shoji, Yasuhiro; Yokota, Yuui; Ohashi, Yuji; Yoshikawa, Akira

    2017-03-01

    Effects of Mg co-doping on scintillation properties of Ce:Lu3(Ga,Al)5O12 (LGAG) were investigated. Mg 200 ppm co-doped Ce:LGAG single crystals were prepared by micro pulling down method. Absorption and radioluminescence spectra were measured together with several other scintillation characteristics, namely the scintillation decay and light yield to reveal the effect of Mg co-doping. Ce4+ charge transfer absorption was observed below 340 nm in Mg,Ce:LGAG which is in good agreement with previous reports for other garnet-based crystals. The scintillation decay time showed the tendency to be accelerated and the light yield was enhanced by Mg co-doping.

  7. Crystal growth and spectroscopic performance of large crystalline boules of CsCaI3:Eu scintillator

    NASA Astrophysics Data System (ADS)

    Lindsey, A.; McAlexander, W.; Stand, L.; Wu, Y.; Zhuravleva, M.; Melcher, C. L.

    2015-10-01

    The crystal growth of CsCaI3:Eu with improved quality over prior efforts for use in X-ray and gamma-ray detection applications is reported. Boules were grown using the vertical Bridgman technique in quartz ampoules at 15, 22, and 35 mm diameters. CsCaI3:Eu crystals show evidence of a heavily twinned microstructure likely caused by a solid-solid phase transformation of the crystal during the cooling process. Energy resolution (FWHM) in large and small samples taken from crystalline boules varies between 13% and 4.5% for 662 keV gamma rays indicating volumetric non-uniformity. Scintillation decay time is shown to increase with volume. Proportionality of the light yield of CsCaI3:Eu is reported for the first time.

  8. Improvement of radiopurity level of enriched 116CdWO4 and ZnWO4 crystal scintillators by recrystallization

    NASA Astrophysics Data System (ADS)

    Barabash, A. S.; Belli, P.; Bernabei, R.; Borovlev, Yu. A.; Cappella, F.; Caracciolo, V.; Cerulli, R.; Danevich, F. A.; Incicchitti, A.; Kobychev, V. V.; Konovalov, S. I.; Laubenstein, M.; Mokina, V. M.; Polischuk, O. G.; Safonova, O. E.; Shlegel, V. N.; Tretyak, V. I.; Tupitsyna, I. A.; Umatov, V. I.; Zhdankov, V. N.

    2016-10-01

    As low as possible radioactive contamination of a detector plays a crucial role to improve sensitivity of a double beta decay experiment. The radioactive contamination of a sample of 116CdWO4 crystal scintillator by thorium was reduced by a factor ≈10, down to the level 0.01 mBq/kg (228Th), by exploiting the recrystallization procedure. The total alpha activity of uranium and thorium daughters was reduced by a factor ≈3, down to 1.6 mBq/kg. No change in the specific activity (the total α activity and 228Th) was observed in a sample of ZnWO4 crystal produced by recrystallization after removing ≈0.4 mm surface layer of the crystal.

  9. Study of a prototype high quantum efficiency thick scintillation crystal video-electronic portal imaging device.

    PubMed

    Samant, Sanjiv S; Gopal, Arun

    2006-08-01

    Image quality in portal imaging suffers significantly from the loss in contrast and spatial resolution that results from the excessive Compton scatter associated with megavoltage x rays. In addition, portal image quality is further reduced due to the poor quantum efficiency (QE) of current electronic portal imaging devices (EPIDs). Commercial video-camera-based EPIDs or VEPIDs that utilize a thin phosphor screen in conjunction with a metal buildup plate to convert the incident x rays to light suffer from reduced light production due to low QE (<2% for Eastman Kodak Lanex Fast-B). Flat-panel EPIDs that utilize the same luminescent screen along with an a-Si:H photodiode array provide improved image quality compared to VEPIDs, but they are expensive and can be susceptible to radiation damage to the peripheral electronics. In this article, we present a prototype VEPID system for high quality portal imaging at sub-monitor-unit (subMU) exposures based on a thick scintillation crystal (TSC) that acts as a high QE luminescent screen. The prototype TSC system utilizes a 12 mm thick transparent CsI(Tl) (thallium-activated cesium iodide) scintillator for QE=0.24, resulting in significantly higher light production compared to commercial phosphor screens. The 25 X 25 cm2 CsI(Tl) screen is coupled to a high spatial and contrast resolution Video-Optics plumbicon-tube camera system (1240 X 1024 pixels, 250 microm pixel width at isocenter, 12-bit ADC). As a proof-of-principle prototype, the TSC system with user-controlled camera target integration was adapted for use in an existing clinical gantry (Siemens BEAMVIEW(PLUS)) with the capability for online intratreatment fluoroscopy. Measurements of modulation transfer function (MTF) were conducted to characterize the TSC spatial resolution. The measured MTF along with measurements of the TSC noise power spectrum (NPS) were used to determine the system detective quantum efficiency (DQE). A theoretical expression of DQE(0) was developed

  10. SCINTILLATION SPECTROMETER

    DOEpatents

    Bell, P.R.; Francis, J.E.

    1960-06-21

    A portable scintillation spectrometer is described which is especially useful in radio-biological studies for determining the uptake and distribution of gamma -emitting substances in tissue. The spectrometer includes a collimator having a plurality of apertures that are hexagonal in cross section. Two crystals are provided: one is activated to respond to incident rays from the collimator; the other is not activated and shields the first from external radiation.

  11. Measurements of the scintillation time constants of inorganic crystals for the development of a triple-Phoswich detector for high-energy X-ray quanta

    NASA Astrophysics Data System (ADS)

    Michelis, Thilo

    1987-04-01

    A setup for the measurement of the rise time distribution of pulses measured by a triple-Phoswich detector that is planned as component of an imaging system of a rotation-modulation telescope (RMT) was built. The principles and characteristics of scintillation crystals, scintillation detectors, and RMT's are outlined. Measurements on CsT(Tl) test crystals show a strong dependence of rise time distribution on Tl-concentration, and a clear dependence on temperature. A system for optimum light collection was developed for a Phoswich detector. The scintillation crystals NaJ(Tl) and CsJ(Na) are very suitable for a strip Phoswich. Proposals for a triple-Phoswich as detector for an RMT are given.

  12. Rare-Earth Tri-Halide Methanol-Adduct Single-Crystal Scintillators for Gamma Ray and Neutron Detection - 8/17/09

    SciTech Connect

    Boatner, Lynn A; Wisniewski, D.; Neal, John S; Bell, Zane W; Ramey, Joanne Oxendine; Kolopus, James A; Chakoumakos, Bryan C; Custelcean, Radu; Wisniewska, Monika; Peña, K. E.

    2009-01-01

    Cerium activated rare-earth tri- halides represent a well-known family of high performance inorganic rare-earth scintillators - including the high-light-yield, high-energy-resolution scintillator, cerium-doped lanthanum tribromide. These hygroscopic inorganic rare-earth halides are currently grown as single crystals from the melt - either by the Bridgman or Czochralski techniques slow and expensive processes that are frequently characterized by severe cracking of the material due to anisotropic thermal stresses and cleavage effects. We have recently discovered a new family of cerium-activated rare-earth metal organic scintillators consisting of tri-halide methanol adducts of cerium and lanthanum namely CeCl3(CH3OH)4 and LaBr3(CH3OH)4:Ce. These methanol-adduct scintillator materials can be grown near room temperature from a methanol solution, and their high solubility is consistent with the application of the rapid solution growth methods that are currently used to grow very large single crystals of potassium dihydrogen phosphate. The structures of these new rare-earth metal-organic scintillating compounds were determined by single crystal x-ray refinements, and their scintillation response to both gamma rays and neutrons, as presented here, was characterized using different excitation sources. Tri-halide methanol-adduct crystals activated with trivalent cerium apparently represent the initial example of a solution-grown rare-earth metal-organic molecular scintillator that is applicable to gamma ray, x-ray, and fast neutron detection.

  13. Search for long-lived superheavy eka-tungsten with radiopure ZnWO4 crystal scintillator

    NASA Astrophysics Data System (ADS)

    Belli, P.; Bernabei, R.; Cappella, F.; Cerulli, R.; Danevich, F. A.; Denisov, V. Yu; d'Angelo, A.; Incicchitti, A.; Kobychev, V. V.; Poda, D. V.; Polischuk, O. G.; Tretyak, V. I.

    2015-08-01

    The data collected with a radioactively pure ZnWO4 crystal scintillator (699 g) in low background measurements during 2130 h at the underground (3600 m w.e.) Laboratori Nazionali del Gran Sasso (INFN, Italy) were used to set a limit on possible concentration of superheavy eka-W (seaborgium Sg, Z = 106) in the crystal. Assuming that one of the daughters in a chain of decays of the initial Sg nucleus decays with emission of high energy α particle ({{Q}α }\\gt 8 MeV) and analyzing the high energy part of the measured α spectrum, the limit N(Sg)/N(W) \\lt 5.5× {{10}-14} atoms/atom at 90% C.L. was obtained (for Sg half-life of 109 yr). In addition, a limit on the concentration of eka-Bi was set by analysing the data collected with a large BGO scintillation bolometer in an experiment performed by another group (Cardani et al 2012 JINST 7 P10022): N(eka-Bi)/N(Bi) \\lt 1.1× {{10}-13} atoms/atom with 90% C.L. Both the limits are comparable with those obtained in recent experiments which instead look for spontaneous fission of superheavy elements or use the accelerator mass spectrometry.

  14. Luminescence and scintillation timing characteristics of (LuxGd2-x)SiO5:Ce single crystals

    NASA Astrophysics Data System (ADS)

    Yawai, Nattasuda; Chewpraditkul, Warut; Sakthong, Ongsa; Chewpraditkul, Weerapong; Wantong, Kriangkrai; Szczesniak, Tomasz; Swiderski, Lukasz; Moszynski, Marek; Sidletskiy, Oleg

    2017-02-01

    The luminescence and scintillation characteristics of cerium-doped lutetium-gadolinium orthosilicate (LuxGd2-xSiO5:Ce; x=0, 0.8, 1.8) single crystals were investigated. At 662 keV γ-rays, the light yield of 29,800±3000 ph MeV-1 obtained for Lu1.8Gd0.2SiO5:Ce is higher than that of 20,200±2000 and 11,800±1200 ph MeV-1 obtained for Lu0.8Gd1.2SiO5:Ce and Gd2SiO5:Ce, respectively. The fast component decay time of 32, 18 and 17 ns was measured in the scintillation decay of Gd2SiO5:Ce, Lu0.8Gd1.2SiO5:Ce and Lu1.8Gd0.2SiO5:Ce, respectively. The coincidence time spectra for 511 keV annihilation quanta were measured in reference to a fast BaF2 detector and time resolution was discussed in terms of a number of photoelectrons and decay time of the fast component. The mass attenuation coefficient for studied crystals at 60 and 662 keV γ-rays was also evaluated and discussed.

  15. Crystal structure, electronic structure, temperature-dependent optical and scintillation properties of CsCe2Br7

    DOE PAGES

    Wu, Yuntao; Shi, Hongliang; Chakoumakos, Bryan C.; ...

    2015-10-05

    CsCe2Br7 is a self-activated inorganic scintillator that shows promising performance, but the understanding of the important structure-property relationships is lacking. In this work, we conduct a comprehensive study on CCsCe2Br7. The crystal structure of CsCe2Br7 is refined using single crystal X-ray study for the first time. It crystallizes into the orthorhombic crystal system with Pmnb space group. Its electronic structure is revealed by Density Functional Theory (DFT) calculations. Two cerium emission centers are identified and the energy barriers related to the thermal quenching to 4f ground states of Ce3+ for these two Ce centers are evaluated. CsCe2Br7 single crystal hasmore » better light yield and energy resolution than CsCe2Cl7, but with an additional slow decay component of 1.7 s. The existence of a deep trap with a depth of 0.9 eV in CsCe2Cl7 contributes to its higher afterglow level in comparison to that of CsCe2Br7. The most possible point defects in CsCe2Cl7 and CsCe2Br7 are proposed by considering the vapour pressure in the growth atmosphere upon melting point.« less

  16. An algorithm for automatic crystal identification in pixelated scintillation detectors using thin plate splines and Gaussian mixture models.

    PubMed

    Schellenberg, Graham; Stortz, Greg; Goertzen, Andrew L

    2016-02-07

    A typical positron emission tomography detector is comprised of a scintillator crystal array coupled to a photodetector array or other position sensitive detector. Such detectors using light sharing to read out crystal elements require the creation of a crystal lookup table (CLUT) that maps the detector response to the crystal of interaction based on the x-y position of the event calculated through Anger-type logic. It is vital for system performance that these CLUTs be accurate so that the location of events can be accurately identified and so that crystal-specific corrections, such as energy windowing or time alignment, can be applied. While using manual segmentation of the flood image to create the CLUT is a simple and reliable approach, it is both tedious and time consuming for systems with large numbers of crystal elements. In this work we describe the development of an automated algorithm for CLUT generation that uses a Gaussian mixture model paired with thin plate splines (TPS) to iteratively fit a crystal layout template that includes the crystal numbering pattern. Starting from a region of stability, Gaussians are individually fit to data corresponding to crystal locations while simultaneously updating a TPS for predicting future Gaussian locations at the edge of a region of interest that grows as individual Gaussians converge to crystal locations. The algorithm was tested with flood image data collected from 16 detector modules, each consisting of a 409 crystal dual-layer offset LYSO crystal array readout by a 32 pixel SiPM array. For these detector flood images, depending on user defined input parameters, the algorithm runtime ranged between 17.5-82.5 s per detector on a single core of an Intel i7 processor. The method maintained an accuracy above 99.8% across all tests, with the majority of errors being localized to error prone corner regions. This method can be easily extended for use with other detector types through adjustment of the initial

  17. An algorithm for automatic crystal identification in pixelated scintillation detectors using thin plate splines and Gaussian mixture models

    NASA Astrophysics Data System (ADS)

    Schellenberg, Graham; Stortz, Greg; Goertzen, Andrew L.

    2016-02-01

    A typical positron emission tomography detector is comprised of a scintillator crystal array coupled to a photodetector array or other position sensitive detector. Such detectors using light sharing to read out crystal elements require the creation of a crystal lookup table (CLUT) that maps the detector response to the crystal of interaction based on the x-y position of the event calculated through Anger-type logic. It is vital for system performance that these CLUTs be accurate so that the location of events can be accurately identified and so that crystal-specific corrections, such as energy windowing or time alignment, can be applied. While using manual segmentation of the flood image to create the CLUT is a simple and reliable approach, it is both tedious and time consuming for systems with large numbers of crystal elements. In this work we describe the development of an automated algorithm for CLUT generation that uses a Gaussian mixture model paired with thin plate splines (TPS) to iteratively fit a crystal layout template that includes the crystal numbering pattern. Starting from a region of stability, Gaussians are individually fit to data corresponding to crystal locations while simultaneously updating a TPS for predicting future Gaussian locations at the edge of a region of interest that grows as individual Gaussians converge to crystal locations. The algorithm was tested with flood image data collected from 16 detector modules, each consisting of a 409 crystal dual-layer offset LYSO crystal array readout by a 32 pixel SiPM array. For these detector flood images, depending on user defined input parameters, the algorithm runtime ranged between 17.5-82.5 s per detector on a single core of an Intel i7 processor. The method maintained an accuracy above 99.8% across all tests, with the majority of errors being localized to error prone corner regions. This method can be easily extended for use with other detector types through adjustment of the initial

  18. Bridgman Growth of Large SrI2:Eu2+ Single Crystals: A High-performance Scintillator for Radiation Detection Applications

    SciTech Connect

    Boatner, Lynn A; Ramey, Joanne Oxendine; Kolopus, James A; Hawrami, Rastgo; Higgins, William; Van Loef, Edgar; Glodo, J.; Shah, Kanai; Bhattacharya, P.; Tupitsyn, E; Groza, Michael; Burger, Arnold

    2013-01-01

    Single-crystal strontium iodide (SrI2) doped with relatively high levels (e.g., 3 - 6 %) of Eu2+ exhibits characteristics that make this material superior, in a number of respects, to other scintillators that are currently used for radiation detection. Specifically, SrI2:Eu2+ has a light yield that is significantly higher than LaBr3:Ce3+ -a currently employed commercial high-performance scintillator. Additionally, SrI2:Eu2+ is characterized by an energy resolution as high as 2.6% at the 137Cs gamma-ray energy of 662 keV, and there is no radioactive component in SrI2:Eu2+ - unlike LaBr3:Ce3+ that contains 138La. The Ce3+-doped LaBr3 decay time is, however, faster (30 nsec) than the 1.2 sec decay time of SrI2:Eu2+. Due to the relatively low melting point of strontium iodide (~515 oC), crystal growth can be carried out in quartz crucibles by the vertical Bridgman technique. Materials-processing and crystal-growth techniques that are specific to the Bridgman growth of europium-doped strontium iodide scintillators are described here. These techniques include the use of a porous quartz frit to physically filter the molten salt from a quartz antechamber into the Bridgman growth crucible and the use of a bent or bulb grain selector design to suppress multiple grain growth. Single crystals of SrI2:Eu2+ scintillators with good optical quality and scintillation characteristics have been grown in sizes up to 5.0 cm in diameter by applying these techniques. Other aspects of the SrI2:Eu2+ crystal-growth methods and of the still unresolved crystal-growth issues are described here.

  19. Comparative Characterization Study of a LaBr3(Ce) Scintillation Crystal in Two Surface Wrapping Scenarios: Absorptive and Reflective

    PubMed Central

    Aldawood, Saad; Castelhano, Ines; Gernhäuser, Roman; Van Der Kolff, Hugh; Lang, Christian; Liprandi, Silvia; Lutter, Rudolf; Maier, Ludwig; Marinšek, Tim; Schaart, Dennis R.; Parodi, Katia; Thirolf, Peter G.

    2015-01-01

    The properties of a 50 mm × 50 mm × 30 mm monolithic LaBr3:Ce scintillator crystal coupled to a position-sensitive multi-anode photomultiplier (PMT, Hamamatsu H9500), representing the absorbing detector of a Compton camera under study for online ion (proton) beam range verification in hadron therapy, was evaluated in combination with either absorptive or reflective crystal surface coating. This study covered an assessment of the energy and position-dependent energy resolution, exhibiting a factor of 2.5–3.5 improvement for the reflectively wrapped crystal at 662 keV. The spatial dependency was investigated using a collimated 137Cs source, showing a steep degradation of the energy resolution at the edges and corners of the absorptively wrapped crystal. Furthermore, the time resolution was determined to be 273 ps (FWHM) and 536 ps (FWHM) with reflective and absorptive coating, respectively, using a 60Co source. In contrast, the light spread function (LSF) of the light amplitude distribution on the PMT segments improved for the absorptively wrapped detector. Both wrapping modalities showed almost no differences in the energy-dependent photopeak detection efficiency. PMID:26697405

  20. Investigation of crystal surface finish and geometry on single LYSO scintillator detector performance for depth-of-interaction measurement with silicon photomultipliers

    NASA Astrophysics Data System (ADS)

    Bircher, Chad; Shao, Yiping

    2012-11-01

    Depth of Interaction (DOI) information can improve quality of reconstructed images acquired from Positron Emission Tomography (PET), especially in high resolution and compact scanners dedicated for breast, brain, or small animal imaging applications. Additionally, clinical scanners with time of flight capability can also benefit from DOI information. One of the most promising methods of determining DOI in a crystal involves reading the signal from two ends of a scintillation crystal, and calculating the signal ratio between the two detectors. This method is known to deliver a better DOI resolution with rough crystals compared to highly polished crystals. However, what is still not well studied is how much of a tradeoff is involved between spatial, energy, temporal, and DOI resolutions as a function of the crystal surface treatment and geometry with the use of Silicon Photomultipliers (SiPM) as the photo detectors. This study investigates the effects of different crystal surface finishes and geometries on energy, timing and DOI resolutions at different crystal depths. The results show that for LYSO scintillators of 1.5×1.5×20 mm3 and 2×2×20 mm3 with their surfaces finished from 0.5 to 30 μm roughness, almost the same energy and coincidence timing resolutions were maintained, around 15% and 2.4 ns, respectively across different crystal depths, while the DOI resolutions were steadily improved from worse than 5 mm to better than 2 mm. They demonstrate that crystal roughness, with proper surface preparing, does not have a significant effect on the energy and coincidence timing resolutions in the crystals examined, and there does not appear to be a tradeoff between improving DOI resolution and degrading other detector performances. These results will be valuable to guide the selection of crystal surface conditions for developing a DOI measurable PET detector with a full array of LYSO scintillators coupled to SiPM arrays.

  1. Investigation of Crystal Surface Finish and Geometry on Single LYSO Scintillator Detector Performance for Depth-of-Interaction Measurement with Silicon Photomultipliers.

    PubMed

    Bircher, Chad; Shao, Yiping

    2012-11-21

    Depth of Interaction (DOI) information can improve quality of reconstructed images acquired from Positron Emission Tomography (PET), especially in high resolution and compact scanners dedicated for breast, brain, or small animal imaging applications. Additionally, clinical scanners with time of flight capability can also benefit from DOI information. One of the most promising methods of determining DOI in a crystal involves reading the signal from two ends of a scintillation crystal, and calculating the signal ratio between the two detectors. This method is known to deliver a better DOI resolution with rough crystals compared to highly polished crystals. However, what is still not well studied is how much of a tradeoff is involved between spatial, energy, temporal, and DOI resolutions as a function of the crystal surface treatment and geometry with the use of Silicon Photomultipliers (SiPM) as the photo detectors. This study investigates the effects of different crystal surface finishes and geometries on energy, timing and DOI resolutions at different crystal depths. The results show that for LYSO scintillators of 1.5×1.5×20 mm(3) and 2×2×20 mm(3) with their surfaces finished from 0.5 to 30 micron roughness, almost the same energy and coincidence timing resolutions were maintained, around 15% and 2.4 ns respectively across different crystal depths, while the DOI resolutions were steadily improved from worse than 5 mm to better than 2 mm. They demonstrate that crystal roughness, with proper surface preparing, does not have a significant effect on the energy and coincidence timing resolutions in the crystals examined, and there does not appear to be a tradeoff between improving DOI resolution and degrading other detector performances. These results will be valuable to guide the selection of crystal surface conditions for developing a DOI measurable PET detector with a full array of LYSO scintillators coupled to SiPM arrays.

  2. Investigations of Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} single crystal as a scintillator

    SciTech Connect

    Zhang, Zhi-Jun; Hu, Guan-Qin; Wang, Hong; Zhu, Lin-Lin; Zhao, Jing-Tai

    2014-04-01

    Highlights: • Eu{sup 2+}-activated Ba{sub 3}BP{sub 3}O{sub 12} single crystals have been grown by the top-seeded solution growth method (TSSG) for the first time. • Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} single crystal exhibits wide transparency in the wavelength range from 250 to 700 nm. • Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} single crystal shows high overall scintillation efficiency (1.8 times of BGO) and moderate decay time (860 ns). - Abstract: Single crystals of Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} with high optical quality have been grown by the top-seeded solution growth (TSSG) method using BPO{sub 4}–NaF mixture as the flux. Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} single crystal exhibits wide transparency in the wavelength range from 250 to 700 nm, and shows a broad emission band in the wavelength range of 350–650 nm when excited by X-ray radiation. The overall scintillation efficiency is about 1.8 times of that of BGO crystal under the same conditions. Its room temperature fluorescence decay curve exhibits a single-exponent shape with decay time of about 860 ns. It is worth noting that Ba{sub 3}BP{sub 3}O{sub 12}:Eu{sup 2+} single crystal may be of great interest for applications in the field of scintillation materials considering its scintillation properties, as well as the good chemical stability.

  3. Improvement of the growth of Li4SiO4 single crystals for neutron detection and their scintillation and luminescence properties

    NASA Astrophysics Data System (ADS)

    Pejchal, Jan; Babin, Vladimir; Beitlerova, Alena; Kurosawa, Shunsuke; Yokota, Yuui; Yoshikawa, Akira; Nikl, Martin

    2017-01-01

    We have investigated Li4SiO4 scintillation crystals for their possible application in neutron detection due to high Li content and low density of 2.35 g/cm3. The micro-pulling-down method employing the Ir crucible and afterheater was optimized for crystal growth of Li4SiO4 taking into account the Li evaporation. To grow high-quality crack-free single crystals, the heating power was increased to establish milder temperature gradient, thicker meniscus, smaller crystal diameter and resulting smaller stress in the as-grown crystals. The undoped, Ti-, Cr-, and Al- doped crystals were prepared and studied. Radioluminescence measurements under X-ray excitation showed quite high overall scintillation efficiency of the Ti-doped sample reaching as high as 250% of that of Bi4Ge3O12 reference scintillator. The emission spectrum was dominated by one broad band peaking at 350 nm related to Ti4+ impurity. Reasonable light yield of 10000 photons/neutron was found. However, its long decay time of 54 μs might be a limitation especially for high counting rate applications. The overall scintillation efficiency of the Cr3+ sample was much lower and the spectrum shows one broad peak at 463 nm which does not correspond to Cr3+ luminescence. The radioluminescence spectrum of the Al-doped sample resembled to that of the Ti-doped one, just its magnitude is considerably lower, which was explained by Ti contamination. Peculiarities and optimization of crystal growth and a preliminary sketch of luminescence mechanisms and dopant incorporation are discussed.

  4. Time walk correction for TOF-PET detectors based on a monolithic scintillation crystal coupled to a photosensor array

    NASA Astrophysics Data System (ADS)

    Vinke, R.; Löhner, H.; Schaart, D. R.; van Dam, H. T.; Seifert, S.; Beekman, F. J.; Dendooven, P.

    2010-09-01

    When optimizing the timing performance of a time-of-flight positron emission tomography (TOF-PET) detector based on a monolithic scintillation crystal coupled to a photosensor array, time walk as a function of annihilation photon interaction location inside the crystal needs to be considered. In order to determine the 3D spatial coordinates of the annihilation photon interaction location, a maximum likelihood estimation algorithm was developed, based on a detector characterization by a scan of a 511 keV photon beam across the front and one of the side surfaces of the crystal. The time walk effect was investigated using a 20 mm×20 mm×12 mm LYSO crystal coupled to a fast 4×4 multi-anode photomultiplier tube (MAPMT). In the plane parallel to the photosensor array, a spatial resolution of 2.4 mm FWHM is obtained. In the direction perpendicular to the MAPMT (depth-of-interaction, DOI), the resolution ranges from 2.3 mm FWHM near the MAPMT to 4 mm FWHM at a distance of 10 mm. These resolutions are uncorrected for the ˜1 mm beam diameter. A coincidence timing resolution of 358 ps FWHM is obtained in coincidence with a BaF 2 detector. A time walk depending on the 3D annihilation photon interaction location is observed. Throughout the crystal, the time walk spans a range of 100 ps. Calibration of the time walk vs. interaction location allows an event-by-event correction of the time walk.

  5. Crystal growth and optical properties of indium doped LiCaAlF6 scintillator single crystals

    NASA Astrophysics Data System (ADS)

    Tanaka, Chieko; Yokota, Yuui; Kurosawa, Shunsuke; Yamaji, Akihiro; Jary, Vitezslav; Babin, Vladimir; Pejchal, Jan; Ohashi, Yuji; Kamada, Kei; Nikl, Martin; Yoshikawa, Akira

    2017-03-01

    The In-doped LiCaAlF6 [In:LiCAF] single crystals were grown by the micro-pulling-down (μ-PD) method, and the phases, chemical compositions, transmittance and radioluminescence spectra were investigated. All the grown crystals showed high transparency and single phase of LiCAF without visible cracks and inclusions except for the end part of In2%:LiCAF crystal which included the impurity phase. In the radioluminescence spectra of the In:LiCAF crystals under X-ray irradiation, the emission peak around 750 nm was revealed.

  6. Assessing the performance under ionising radiation of lead tungstate scintillators for EM calorimetry in the CLAS12 Forward Tagger

    NASA Astrophysics Data System (ADS)

    Fegan, S.; Auffray, E.; Battaglieri, M.; Buchanan, E.; Caiffi, B.; Celentano, A.; Colaneri, L.; D`Angelo, A.; De Vita, R.; Dormenev, V.; Fanchini, E.; Lanza, L.; Novotny, R. W.; Parodi, F.; Rizzo, A.; Sokhan, D.; Tarasov, I.; Zonta, I.

    2015-07-01

    The well-established technology of electromagnetic calorimetry using Lead Tungstate crystals has recently seen an upheaval, with the closure of one of the most experienced large-scale suppliers of such crystals, the Bogoroditsk Technical Chemical Plant (BTCP), which was instrumental in the development of mass production procedures for PWO-II, the current benchmark for this scintillator. Obtaining alternative supplies of Lead Tungstate crystals matching the demanding specifications of contemporary calorimeter devices now presents a significant challenge to detector research and development programmes. In this paper we describe a programme of assessment carried out for the selection, based upon the performance under irradiation, of Lead Tungstate crystals for use in the Forward Tagger device, part of the CLAS12 detector in Hall B at Jefferson Lab. The crystals tested were acquired from SICCAS, the Shanghai Institute of Ceramics, Chinese Academy of Sciences. The tests performed are intended to maximise the performance of the detector within the practicalities of the crystal manufacturing process. Results of light transmission, before and after gamma ray irradiation, are presented and used to calculate dk, the induced radiation absorption coefficient, at 420 nm, the peak of the Lead Tungstate emission spectrum. Results for the SICCAS crystals are compared with identical measurements carried out on Bogoroditsk samples, which were acquired for the Forward Tagger development program before the closure of the facility. Also presented are a series of tests performed to determine the feasibility of recovering radiation damage to the crystals using illumination from an LED, with such illumination available in the Forward Tagger from a light monitoring system integral to the detector.

  7. Growth of 2 Inch Eu-doped SrI2 single crystals for scintillator applications

    NASA Astrophysics Data System (ADS)

    Yoshikawa, Akira; Shoji, Yasuhiro; Yokota, Yuui; Kurosawa, Shunsuke; Hayasaka, Shoki; Chani, Valery I.; Ito, Tomoki; Kamada, Kei; Ohashi, Yuji; Kochurikhin, Vladimir

    2016-10-01

    A vertical Bridgman (VB) crystal growth process was established using modified micro-pulling-down (μ-PD) crystal growth system with a removable chamber that was developed for the growth of deliquescent halide single crystals because conventional μ-PD method does not allow growth of large bulk single crystals. Eu:SrI2 crystals were grown from the melt of (Sr0.98Eu0.02)I2 composition using carbon crucibles. Undoped μ-PD SrI2 crystals were used as seeds that were affixed to the bottom of the crucible. All the preparations preceding the growths and the hot zone assembling were performed in a glove box with Ar gas. Then the removable chamber was taken out of the glove box, attached to the μ-PD system, connected with a Turbo Molecular pump, and evacuated down to 10-4 Pa at 300 °C. After the baking procedure, high purity Ar gas (6N) was injected into the chamber. The crucible was heated by a high frequency induction coil up to the melting point of Eu:SrI2. After melting the starting materials, the crucible was displaced in downward direction for the crystal growth and then cooled down to room temperature. Thus, 2 in. and crack-free Eu:SrI2 bulk crystals were produced. The crystals had high transparency and did not contain any visible inclusions. The crystals were cut and polished in the glove box and then sealed in an aluminum container with an optical window for characterization. The details of the crystal growth are discussed.

  8. Designing and constructing of a two scintillator crystal rotatable telescope for muon flux variation studies

    NASA Astrophysics Data System (ADS)

    Alghamdi, Abdullrahman; Maghrabi, Abdullrahman H.; Almutari, Mohammed M.

    2014-07-01

    A rotatable muon detection telescope with two layers of scintillators was designed and constructed at the physics detector laboratory at KACST, Saudi Arabia. The objective of this system is to study the zenith angle dependence of high energy cosmic ray muons. The system has the flexibility to rotate in all directions to cover the zenith angle from 0- 900 for muon distribution studies, as well as the azimuth angle from 0-3590 to observe the geomagnetic field effects on it. In this paper, the designing and the construction works as well as the calibration procedures for the detection system will be given. Some of the preliminarily results and some of the future experiments and possible modifications will be outlined.

  9. Search for double beta processes in {sup 106}Cd with enriched {sup 106}CdWO{sub 4} crystal scintillator in coincidence with four crystals HPGe detector

    SciTech Connect

    Danevich, F. A. Chernyak, D. M.; Mokina, V. M.; Belli, P.; Bernabei, R.; D’Angelo, S.; Brudanin, V. B.; Cappella, F.; Caracciolo, V.; Cerulli, R.; Laubenstein, M.; Incicchitti, A.; Poda, D. V.; Polischuk, O. G.; Tretyak, V. I.; Tupitsyna, I. A.

    2015-10-28

    A radiopure cadmium tungstate crystal scintillator, enriched in {sup 106}Cd ({sup 106}CdWO{sub 4}), was used to search for double beta decay processes in {sup 106}Cd in coincidence with an ultra-low background set-up containing four high purity germanium (HPGe) detectors in a single cryostat. The experiment has been completed after 13085 h of data taking. New improved limits on most of the double beta processes in {sup 106}Cd have been set on the level of 10{sup 20}−10{sup 21} yr. Tn particular, the half-life limit on the two neutrino electron capture with positron emission, T{sub 1/2} ≥ 1.8 × 10{sup 21} yr, reached the region of theoretical predictions.

  10. A comparison of the use of sodium iodide and lanthanum bromide scintillation crystals for airborne surveys

    NASA Astrophysics Data System (ADS)

    Bailey, Derek M.

    The Environmental Protection Agency (EPA) Aerial Spectral Environmental Collection Technology (ASPECT) program performs aerial radiological and chemical characterization of geographical regions of interest. Airborne surveys are performed to characterize environmental radionuclide content, for mineral exploration, as well as for emergency scenarios such as major releases or lost sources. Two radiological detection systems are used by the ASPECT team for gamma-ray detection and characterization: lanthanum bromide [LaBr 3(Ce)] and sodium iodide [NaI(Tl)] scintillation systems. An aerial survey of a uranium mine in the western United States was performed using both NaI(Tl) and LaBr3(Ce) detection systems. Analyses of the survey data were performed with RadAssist software and applying International Atomic Energy Agency (IAEA) airborne gamma ray mapping guidelines. The data for the survey were corrected for cross-over, which is spectral interference from higher energy photons as a result of Compton scattering, height attenuation, cosmic ray contribution to signal, and Radon contribution to signal. Two radiation survey contours were generated from each discrete data set. Based on analysis of the uranium mine survey results, LaBr3(Ce) produced a product comparable to that of NaI(Tl). The LaBr3(Ce) detection system contained 1/16th the scintillating volume and had a total system weight that was 1/4th that of the NaI(Tl) system. LaBr3(Ce) demonstrated a clear advantage over NaI(Tl) detectors in system mobility, and weight factors in airborne gamma ray spectroscopy.

  11. SCINTILLATION EXPOSURE RATE DETECTOR

    DOEpatents

    Spears, W.G.

    1960-11-01

    A radiation detector for gamma and x rays is described. The detector comprises a scintillation crystal disposed between a tantalum shield and the input of a photomultiplier tube, the crystal and the shield cooperating so that their combined response to a given quantity of radiation at various energy levels is substantially constant.

  12. A deeper insight into (Lu,Y)AG:Pr scintillator crystals

    NASA Astrophysics Data System (ADS)

    Drozdowski, W.; Wojtowicz, A. J.; Brylew, K.; Łachmański, W.; Talik, E.; Szubka, M.; Kusz, J.; Guzik, A.; Balin, K.; Kisielewski, J.; Świrkowicz, M.; Pajączkowska, A.

    2017-02-01

    Interior of Czochralski-grown (Lu,Y)AG:Pr crystals has been examined by means of several techniques, such as X-Ray Photoelectron Spectroscopy, X-Ray Diffraction, Time-of-Flight Secondary Ion Mass Spectrometry, and magnetic susceptibility measurements. Additionally, their luminescence has been monitored at various combinations of a double-beam (X-ray/IR) excitation.

  13. Crystal structure and thermal expansion of a CsCe2Cl7 scintillator

    DOE PAGES

    Zhuravleva, M.; Lindsey, A.; Chakoumakos, B. C.; ...

    2015-04-06

    Here we used single-crystal X-ray diffraction data to determine crystal structure of CsCe2Cl7. It crystallizes in a P1121/b space group with a = 19.352(1) Å, b = 19.352(1) Å, c = 14.838(1) Å, γ = 119.87(2) ° , and V = 4818.6(5) Å3. Differential scanning calorimetry measurements combined with the structural evolution of CsCe2Cl7 via X-ray diffractometry over a temperature range from room temperature to the melting point indicates no obvious intermediate solid-solid phase transitions. The anisotropy in the average linear coefficient of thermal expansion of the a axis (21.3 10-6/ °C) with respect to the b and c axesmore » (27.0 10-6/ °C) was determined through lattice parameter refinement of the temperature dependent diffraction patterns. Lastly, these findings suggest that the reported cracking behavior during melt growth of CsCe2Cl7 bulk crystals using conventional Bridgman and Czochralski techniques may be largely attributed to the anisotropy in thermal expansion.« less

  14. Search for double beta decay of 116Cd with enriched 116CdWO4 crystal scintillators (Aurora experiment)

    NASA Astrophysics Data System (ADS)

    Danevich, F. A.; Barabash, A. S.; Belli, P.; Bernabei, R.; Cappella, F.; Caracciolo, V.; Cerulli, R.; Chernyak, D. M.; d'Angelo, S.; Incicchitti, A.; Kobychev, V. V.; Konovalov, S. I.; Laubenstein, M.; Mokina, V. M.; Poda, D. V.; Polischuk, O. G.; Shlegel, V. N.; Tretyak, V. I.; Umatov, V. I.

    2016-05-01

    The Aurora experiment to investigate double beta decay of 116 Cd with the help of 1.162 kg cadmium tungstate crystal scintillators enriched in 116 Cd to 82% is in progress at the Gran Sasso Underground Laboratory. The half-life of 116 Cd relatively to the two neutrino double beta decay is measured with the highest up-to-date accuracy T1/2 = (2.62 ± 0.14) × 1019 yr. The sensitivity of the experiment to the neutrinoless double beta decay of 116 Cd to the ground state of 116 Sn is estimated as T1/2 ≥ 1.9 × 1023 yr at 90% CL, which corresponds to the effective Majorana neutrino mass limit (mv) ≤ (1.2 — 1.8) eV. New limits are obtained for the double beta decay of 116 Cd to the excited levels of 116 Sn, and for the neutrinoless double beta decay with emission of majorons.

  15. Electron spin resonance study of self-trapped holes in CdWO{sub 4} scintillator crystals

    SciTech Connect

    Laguta, V. V.; Nikl, M.; Rosa, J.; Grinyov, B. V.; Nagornaya, L. L.; Tupitsina, I. A.

    2008-11-15

    The self-trapping of holes at oxygen anions was studied by electron spin resonance in UV irradiated CdWO{sub 4} crystals. Analysis of superhyperfine interaction of the holes with {sup 183}W and {sup 111,113}Cd isotopes shows that the self-trapped hole is either delocalized in the space between two energetically equivalent nearest neighbor oxygen ions or tunnels between them. When the temperature increases above 40-50 K the self-trapped holes are thermally liberated and can be retrapped by oxygen ions perturbed by impurity ions. In case of the Nb{sup 5+} or Li{sup +} stabilizing impurities the O{sup -} centers are thermally stable up to 160-170 K. The study of kinetic characteristics of the self-trapped holes suggests that holes leave oxygen ions by thermally assisted tunneling mechanism via two slightly different channels. Corresponding ionization probabilities are defined by the Arrhenius law with an average thermal ionization energy E=90(5) meV. Calculated pre-exponential factors, about 10{sup 5} s{sup -1}, are small, which is consistent with the tunneling mechanism. Thermal stability and kinetic characteristics of the trapped holes are discussed in light of the scintillation and thermoluminescence characteristics of CdWO{sub 4}.

  16. Development of radiopure cadmium tungstate crystal scintillators from enriched {sup 106}Cd and {sup 116}Cd to search for double beta decay

    SciTech Connect

    Danevich, F. A.; Boiko, R. S.; Chernyak, D. M.; Kobychev, V. V.; Kropivyansky, B. N.; Mokina, V. M.; Nikolaiko, A. S.; Poda, D. V.; Podviyanuk, R. B.; Tretyak, V. I.; Barabash, A. S.; Konovalov, S. I.; Umatov, V. I.; Belli, P.; Bernabei, R.; D'Angelo, S.; Brudanin, V. B.; Cappella, F.; Incicchitti, A.; Caracciolo, V.; and others

    2013-08-08

    Cadmium tungstate crystal scintillators enriched in {sup 106}Cd up to 66% ({sup 106}CdWO{sub 4}) and in {sup 116}Cd up to 82% ({sup 116}CdWO{sub 4}) have been developed. The low radioactive contamination of the crystals measured on the level of ≤ 1.5 mBq/kg ({sup 40}K), ≤ 0.005 - 0.012 mBq/kg ({sup 226}Ra), 0.04 - 0.07 mBq/kg ({sup 228}Th) allows to carry out high sensitivity experiments to search for double beta processes in {sup 106}Cd and {sup 116}Cd.

  17. Exploratory growth in the Li2MoO4-MoO3 system for the next crystal generation of heat-scintillation cryogenic bolometers

    NASA Astrophysics Data System (ADS)

    Velázquez, Matias; Veber, Philippe; Moutatouia, Meryem; de Marcillac, Pierre; Giuliani, Andrea; Loaiza, Pia; Denux, Dominique; Decourt, Rodolphe; El Hafid, Hassan; Laubenstein, Matthias; Marnieros, Stefanos; Nones, Claudia; Novati, Valentina; Olivieri, Emiliano; Poda, Denys V.; Zolotarova, Anastasiia S.

    2017-03-01

    In this work, we report on the Czochralski growth of Li2MoO4 crystals up to 230 g for heat-scintillation cryogenic bolometers likely to be used in astroparticle physics and neutron spectroscopy. Their transmission properties, radiopurity levels and detector behavior characterizations were carried out in order to validate the crystal growth process. The melting characteristics, the partition coefficients of a broad range of impurities, the thermal expansion (lattice parameters and dilatometry) and specific heat properties of the crystals were measured, over a broad temperature range for the last two, providing new data likely to be used in crystal growth process numerical simulations. We also investigated the crystal growth of Li4Mo5O17 and determined its melting behavior and specific heat. The physical properties directly relevant to heat-scintillation cryogenic bolometers of Li2MoO4 and Li4Mo5O17 are discussed in the context of the current materials developed for such applications.

  18. Hole capture in PbWO{sub 4}:Mo,La(Y) scintillator crystals

    SciTech Connect

    Laguta, V. V.; Buryi, M.; Nikl, M.; Rosa, J.; Zazubovich, S.

    2011-03-01

    The processes of hole localization in PbWO{sub 4}:Mo,La(Y) single crystals were investigated by electron spin resonance. It was found that the holes created by uv irradiation are trapped at the regular oxygen ions in the vicinity of perturbing defects such as lead vacancies, impurity ions (La,Y), and other lattice imperfections. This leads to a variety of O{sup -} centers which differ in both the thermal stability (from about 160 K up to 240 K) and spectroscopic parameters. The thermal release of such trapped holes and their subsequent recombination with electrons stored at different traps, including (MoO{sub 4}){sup 3-} complexes, are accompanied by the appearance of the thermally stimulated luminescence peaks located at around 190 K and in the 225-250 K range.

  19. A novel scintillation imager with charge-spread discrimination. Analytical models suitable for crystal-arrays

    NASA Astrophysics Data System (ADS)

    Scafè, Raffaele; Pellegrini, Rosanna; Cinti, Maria N.; Puccini, Marco; Pani, Roberto

    2016-10-01

    Present paper describes a method for obtaining the physical quantities characterizing single-events based on fitting experimental 2-D charge-profiles to two analytical models. First results are presented regarding a 10×10 LuYAP:Ce array of 2×2×10 mm3 crystal pixels coupled to a H10966 Hamamatsu 8×8 multi-anode assembly under radio-isotopic irradiations and from self-activity. Results show that a photo multiplier tube with cross plate anode configuration would be preferable than a multi anode one due to uniformity, cost, and connections constraints. Among the results a plot of charge spread Vs. charge is to be cited because it was not yet published in scientific literature.

  20. Optical and scintillation properties of ce-doped (Gd2Y1)Ga2.7Al2.3O12 single crystal grown by Czochralski method

    NASA Astrophysics Data System (ADS)

    Wang, Chao; Wu, Yuntao; Ding, Dongzhou; Li, Huanying; Chen, Xiaofeng; Shi, Jian; Ren, Guohao

    2016-06-01

    Multicomponent garnets, due to their excellent light yield and energy resolution, become one of the most promising scintillators used for homeland security and nuclear non-proliferation applications. This work focuses on the optimization of Ce-doped (Gd,Y)3(Ga,Al)5O12 scintillators using a combination strategy of pre-screening and scale-up. Ce-doped GdxY1-xGayAl5-yO12 (x=1, 2 and y=2, 2.2, 2.5, 2.7, 3) polycrystalline powders were prepared by high-temperature solid state reaction method. The desired garnet phase in all the samples was confirmed using X-ray diffraction measurement. By comparing the radioluminescence intensity, the highest scintillation efficiency was achieved at a component of Gd2Y1Ga2.7Al2.3O12:Ce powders. A (Gd2Y1)Ga2.7Al2.3O12 doped with 1% Ce single crystal with dimensions of Ø35×40 mm was grown by Czochralski method using a <111> oriented seed. Luminescence and scintillation properties were measured. An optical transmittance of 84% was achieved in the concerned wavelength from 500 to 800 nm. Its 5d-4f emission of Ce3+ is at 530 nm. The light yield of a Ce1%: Gd2Y1Ga2.7Al2.3O12 single crystal slab at a size of 5×5×1 mm3 can reach about 65,000±3000 Ph/MeV along with two decay components of 94 and 615 ns under 137Cs source irradiation.

  1. Bridgman crystal growth and spectral properties of Er doped PbWO4 as stimulated Raman crystals

    NASA Astrophysics Data System (ADS)

    Xiong, Wei; Chen, Liang; Guo, Feiyun; Zhou, Yao; Su, Liangbi; Yang, Yan; Yuan, Hui

    2012-06-01

    Several Er doped (0.2 at%, 0.5 at%, and 1.0 at%) PbWO4 single crystals were grown by Bridgman method with the size of Φ20 × 100 mm. The absorption spectra of Er:PWO samples were measured to investigate the spectral properties of Er3+ ions according to Judd-Ofelt theory. The phenomenological intensity parameters Ωλ were fitted to calculate the spectral parameters of several radiative transitions of Er3+ ions, and the possibility of 4I13/2 → 4I15/2 transition at about 1.5 μm of Er3+ ions in PWO crystal was also discussed. The energy transfer from PWO matrix to Er3+ ions was investigated based on the photoluminescence spectra, and the frequency shifting effect of Er3+ ions on PWO crystal was discussed according to the spontaneous Raman spectra. The 1.5 μm fluorescence spectra of different Er:PWO samples were measured under the excitation at 980 nm.

  2. Scintillation characteristics of LiCaAlF6-based single crystals under X-ray excitation

    NASA Astrophysics Data System (ADS)

    Nikl, M.; Bruza, P.; Panek, D.; Vrbova, M.; Mihokova, E.; Mares, J. A.; Beitlerova, A.; Kawaguchi, N.; Fukuda, K.; Yoshikawa, A.

    2013-04-01

    LiCaAlF6-based scintillators are studied under X- and soft gamma-ray excitations. Under nanosecond pulsed soft X-ray laser excitation the scintillation decay is measured with extremely high dynamical resolution and broad time scale. The undoped LiCaAlF6 shows complex temperature dependence of exciton luminescence and tunneling-driven energy transfer process in scintillation decay. In both the Ce and Eu-doped LiCaAlF6 the dominant part of measured scintillation decay is due to prompt recombination of electrons and holes at the doped emission centers. Nevertheless, the measured light yield value is considerably lower with respect to the derived upper limits. Possible origin of its deterioration is discussed.

  3. Study of a Li doped CsI scintillator crystal as a neutron detector

    NASA Astrophysics Data System (ADS)

    Madi Filho, T.; Pereira, M. C. C.; Berretta, J. R.; Cárdenas, J. P. N.

    2015-07-01

    The radiation monitoring system is an important requirement in the premises of a nuclear reactor. A variety of types of radiation (neutrons. gamma. beta and fission products) exist in a reactor. associated to the broad energy spectrum of these radiations. implying the need of detectors to be used in the reactor system and security. as well as radiation monitoring. As the neutron sources are associated to gamma radiation. it is necessary that the neutron detecting system may be capable to discriminate the gamma interference. In our work environment. there are two Nuclear Research Reactors and a neutron irradiator with two AmBe sources (592GBq of Am. each). These conditions warrant the development of new types of detectors. Due to the absence of charge in the neutron. it is necessary to use a converter material that generates radiations capable to produce signals in the detector. Materials with high cross section. like Li or B. are used for this purpose. The CsIcrystal doped with 6Li has been studied. The concentration of the lithium doping element (Li) studied was 10-3M. The detector test was done using an AmBe source (37GBq) and gamma sources. The crystal was coupled to a photomultiplier.

  4. Hole and electron traps in the YAlO{sub 3} single crystal scintillator

    SciTech Connect

    Laguta, V. V.; Nikl, M.; Rosa, J.; Vedda, A.; Mihokova, E.; Blazek, K.

    2009-07-15

    The processes of hole and electron localization in YAlO{sub 3} single crystals were investigated by electron-spin resonance. It was found that holes created by UV or x-ray irradiation are trapped at regular oxygen ions forming two types of O{sup -} hole centers corresponding to hole localization at two inequivalent oxygen ions which are located in Y and Al planes, respectively. The hole can be either autolocalized or additionally stabilized by a defect in the neighborhood of the oxygen ion such as yttrium vacancy or an impurity ion at Y site. This leads to a variety of O{sup -} centers which differ both by thermal stability (from about 14 K up to room temperature) and spectral parameters. Electron-type trapping sites are assigned to Y{sub Al} antisite ions. After trapping an electron they become paramagnetic Y{sub Al}{sup 2+} centers. They are found in several configurations with thermal stability up to above 300 K that enables the radiative recombination of freed holes with such localized electrons and the appearance of thermoluminescence peaks. It is shown that the electron trapped around Y{sub Al} antisite ion is additionally stabilized either by an oxygen vacancy or by a defect at Y site. The yttrium antisite ions in the lattice were directly identified by {sup 89}Y nuclear magnetic resonance.

  5. Test beam results with a sampling calorimeter of cerium fluoride scintillating crystals and tungsten absorber plates for calorimetry at the HL-LHC

    NASA Astrophysics Data System (ADS)

    Becker, R.; Dissertori, G.; Djambazov, L.; Donegà, M.; Dröge, M.; Haller, C.; Horisberger, U.; Lustermann, W.; Nessi-Tedaldi, F.; Quittnat, M.; Pandolfi, F.; Peruzzi, M.; Schönenberger, M.; Cavallari, F.; Dafinei, I.; Diemoz, M.; D`Imperio, G.; del Re, D.; Gelli, S.; Jorda Lope, C.; Meridiani, P.; Micheli, F.; Nuccetelli, M.; Organtini, G.; Paramatti, R.; Pellegrino, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Tabarelli de Fatis, T.; Martelli, A.; Monti, V.; Pastrone, N.; Trapani, P. P.; Candelise, V.; Della Ricca, G.

    2016-07-01

    A sampling calorimeter using cerium fluoride scintillating crystals as active material, interleaved with absorber plates made of tungsten, and read out by wavelength-shifting fibres has been tested with high-energy electron beams at the CERN SPS H4 beam line, as well as with lower-energy beams at the INFN Frascati Beam Test Facility in Italy. Energy resolution studies revealed a low stochastic term (< 10 % /√{ E }). This result, combined with high radiation hardness of the material used, marks this sampling calorimeter as a good candidate for the detectors' forward regions during the high luminosity phase of LHC.

  6. Scintillator material

    DOEpatents

    Anderson, D.F.; Kross, B.J.

    1992-07-28

    An improved scintillator material comprising cerium fluoride is disclosed. Cerium fluoride has been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to known scintillator materials such as thallium-doped sodium iodide, barium fluoride and bismuth germanate. As a result, cerium fluoride is favorably suited for use as a scintillator material in positron emission tomography. 4 figs.

  7. Scintillator material

    DOEpatents

    Anderson, David F.; Kross, Brian J.

    1994-01-01

    An improved scintillator material comprising cerium fluoride is disclosed. Cerium fluoride has been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to known scintillator materials such as thallium-doped sodium iodide, barium fluoride and bismuth germanate. As a result, cerium fluoride is favorably suited for use as a scintillator material in positron emission tomography.

  8. Scintillator material

    DOEpatents

    Anderson, David F.; Kross, Brian J.

    1992-01-01

    An improved scintillator material comprising cerium fluoride is disclosed. Cerium fluoride has been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to known scintillator materials such as thallium-doped sodium iodide, barium fluoride and bismuth germanate. As a result, cerium fluoride is favorably suited for use as a scintillator material in positron emission tomography.

  9. Scintillator material

    DOEpatents

    Anderson, D.F.; Kross, B.J.

    1994-06-07

    An improved scintillator material comprising cerium fluoride is disclosed. Cerium fluoride has been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to known scintillator materials such as thallium-doped sodium iodide, barium fluoride and bismuth germanate. As a result, cerium fluoride is favorably suited for use as a scintillator material in positron emission tomography. 4 figs.

  10. Control of mean ionic radius at Ca site by Sr co-doping for Ce doped LiCaAlF6 single crystals and the effects on optical and scintillation properties

    NASA Astrophysics Data System (ADS)

    Yokota, Yuui; Yamaji, Akihiro; Kurosawa, Shunsuke; Kamada, Kei; Yoshikawa, Akira

    2014-10-01

    Sr co-doped Ce:LiCaAlF6 [Ce:Li(Ca,Sr)AlF6] crystals with various Ca/Sr ratios were grown by a micro-pulling-down (μ-PD) method and effects of Sr co-doping on crystal structure, chemical composition, optical and scintillation properties for Ce:LiCaAlF6 crystals were investigated as a neutron scintillator. High transparent Ce2%:Li(Ca,Sr)AlF6 crystals with 2% and 5% Sr contents were obtained while Ce2%:Li(Ca,Sr)AlF6 crystals with 10% and 20% Sr contents included milky parts in the crystals. a- and c-axis lengths of Ce:Li(Ca,Sr)AlF6 phase systematically increased with an increase of Sr content. In addition to the emission at 284 and 308 nm from Ce3+ ion, emission peaks at 367 nm appeared by Sr co-doping.

  11. Effect of ZnI2 cosolute on quality and performance of γ-CuI ultrafast scintillation crystal grown via evaporation method in acetonitrile solvent

    NASA Astrophysics Data System (ADS)

    Yue, Shuangqiang; Gu, Mu; Liu, Xiaolin; Zhang, Juannan; Huang, Shiming; Liu, Bo; Ni, Chen

    2017-04-01

    γ-CuI single crystal was grown via evaporation method in ZnI2 acetonitrile solvent. The ZnI2 plays a unique role which can not only increase the solubility of CuI in acetonitrile but also introduce the Zn and I ions in the crystal. The γ-CuI crystal grown in ZnI2 acetonitrile is regular and transparent. Its size reaches up to 18 × 11 × 2 mm3 which is larger than that of the crystal grown in pure acetonitrile. In terms of the photoluminescence, the intensity of the emission at 411 nm of the crystal grown with ZnI2 as a cosolute is much higher than that of the crystal grown without ZnI2, which implies that the crystallinity of the crystal can be improved by ZnI2 doping. The X-ray excited luminescence of the crystal shows that the emission at 435 nm can be significantly enhanced and the emission near 680 nm can be suppressed by introducing Zn and I in the natural non-stoichiometry γ-CuI crystal. The nature of the phenomena is discussed. The decay time of the emission at 435 nm similar to that of the emission at 411 nm is faster than the detection limit of the instrument, i.e. less than 1 ns, and the average decay time of the emission near 680 nm is about 183 ns. The results can provide a useful guide to optimize the scintillation properties of γ-CuI single crystal.

  12. Photofraction of a 5 cm x 2 cm BGO scintillator. [bismuth germanate crystal for use in cosmic gamma ray detector

    NASA Technical Reports Server (NTRS)

    Dunphy, P. P.; Forrest, D. J.

    1985-01-01

    The photofraction of a 5.1 cm x 2.0 cm bismuth germanate (BGO) scintillator was measured over a gamma-ray energy range of 0.2 to 6.1 MeV. Several methods, used to minimize the effect of room scattering on the measurement, are discussed. These include a gamma-gamma coincidence technique, a beta-gamma coincidence technique, and the use of sources calibrated with a standard 7.6 cm x 7.6 cm sodium iodide scintillator.

  13. Scintillation Counters

    NASA Astrophysics Data System (ADS)

    Bell, Zane W.

    Scintillators find wide use in radiation detection as the detecting medium for gamma/X-rays, and charged and neutral particles. Since the first notice in 1895 by Roentgen of the production of light by X-rays on a barium platinocyanide screen, and Thomas Edison's work over the following 2 years resulting in the discovery of calcium tungstate as a superior fluoroscopy screen, much research and experimentation have been undertaken to discover and elucidate the properties of new scintillators. Scintillators with high density and high atomic number are prized for the detection of gamma rays above 1 MeV; lower atomic number, lower-density materials find use for detecting beta particles and heavy charged particles; hydrogenous scintillators find use in fast-neutron detection; and boron-, lithium-, and gadolinium-containing scintillators are used for slow-neutron detection. This chapter provides the practitioner with an overview of the general characteristics of scintillators, including the variation of probability of interaction with density and atomic number, the characteristics of the light pulse, a list and characteristics of commonly available scintillators and their approximate cost, and recommendations regarding the choice of material for a few specific applications. This chapter does not pretend to present an exhaustive list of scintillators and applications.

  14. Design and simulation of a novel method for determining depth-of-interaction in a PET scintillation crystal array using a single-ended readout by a multi-anode PMT

    NASA Astrophysics Data System (ADS)

    Ito, Mikiko; Lee, Jae Sung; Park, Min-Jae; Sim, Kwang-Souk; Jong Hong, Seong

    2010-07-01

    PET detectors with depth-of-interaction (DOI) encoding capability allow high spatial resolution and high sensitivity to be achieved simultaneously. To obtain DOI information from a mono-layer array of scintillation crystals using a single-ended readout, the authors devised a method based on light spreading within a crystal array and performed Monte Carlo simulations with individual scintillation photon tracking to prove the concept. A scintillation crystal array model was constructed using a grid method. Conventional grids are constructed using comb-shaped reflector strips with rectangular teeth to isolate scintillation crystals optically. However, the authors propose the use of triangularly shaped teeth, such that scintillation photons spread only in the x-direction in the upper halves of crystals and in the y-direction in lower halves. DOI positions can be estimated by considering the extent of two-dimensional light dispersion, which can be determined from the multiple anode outputs of a position-sensitive PMT placed under the crystal array. In the main simulation, a crystal block consisting of a 29 × 29 array of 1.5 mm × 1.5 mm × 20 mm crystals and a multi-anode PMT with 16 × 16 pixels were used. The effects of crystal size and non-uniform PMT output gain were also explored by simulation. The DOI resolution estimated for 1.5 × 1.5 × 20 mm3 crystals was 2.16 mm on average. Although the flood map was depth dependent, each crystal was well identified at all depths when a corner of the crystal array was irradiated with 511 keV gamma rays (peak-to-valley ratio ~9:1). DOI resolution was better than 3 mm up to a crystal length of 28 mm with a 1.5 × 1.5 mm2 or 2.0 × 2.0 mm2 crystal surface area. The devised light-sharing method allowed excellent DOI resolutions to be obtained without the use of dual-ended readout or multiple crystal arrays.

  15. Design and simulation of a novel method for determining depth-of-interaction in a PET scintillation crystal array using a single-ended readout by a multi-anode PMT.

    PubMed

    Ito, Mikiko; Lee, Jae Sung; Park, Min-Jae; Sim, Kwang-Souk; Hong, Seong Jong

    2010-07-07

    PET detectors with depth-of-interaction (DOI) encoding capability allow high spatial resolution and high sensitivity to be achieved simultaneously. To obtain DOI information from a mono-layer array of scintillation crystals using a single-ended readout, the authors devised a method based on light spreading within a crystal array and performed Monte Carlo simulations with individual scintillation photon tracking to prove the concept. A scintillation crystal array model was constructed using a grid method. Conventional grids are constructed using comb-shaped reflector strips with rectangular teeth to isolate scintillation crystals optically. However, the authors propose the use of triangularly shaped teeth, such that scintillation photons spread only in the x-direction in the upper halves of crystals and in the y-direction in lower halves. DOI positions can be estimated by considering the extent of two-dimensional light dispersion, which can be determined from the multiple anode outputs of a position-sensitive PMT placed under the crystal array. In the main simulation, a crystal block consisting of a 29x29 array of 1.5 mmx1.5 mmx20 mm crystals and a multi-anode PMT with 16x16 pixels were used. The effects of crystal size and non-uniform PMT output gain were also explored by simulation. The DOI resolution estimated for 1.5x1.5x20 mm3 crystals was 2.16 mm on average. Although the flood map was depth dependent, each crystal was well identified at all depths when a corner of the crystal array was irradiated with 511 keV gamma rays (peak-to-valley ratio approximately 9:1). DOI resolution was better than 3 mm up to a crystal length of 28 mm with a 1.5x1.5 mm2 or 2.0x2.0 mm2 crystal surface area. The devised light-sharing method allowed excellent DOI resolutions to be obtained without the use of dual-ended readout or multiple crystal arrays.

  16. Optical and scintillation properties of Ce:(Gd8AE2)(SiO4)6O2 (AE = Mg, Ca, Sr and Ba) crystals

    NASA Astrophysics Data System (ADS)

    Igashira, Takuya; Mori, Masaki; Okada, Go; Kawaguchi, Noriaki; Yanagida, Takayuki

    2017-02-01

    1% Ce-doped and non-doped (Gd8AE2)(SiO4)6O2 (AE = Mg, Ca, Sr and Ba) (denoted as GMS, GCS, GSrS and GBS, respectively) single crystals were grown by the Floating Zone (FZ) method to evaluate their optical and scintillation properties. The Ce:GCS and Ce:GSrS samples exhibited scintillation and photoluminescence (PL) around 400 nm due to the 5d-4f transitions of Ce3+. On the other hand, Ce:GMS and Ce:GBS showed much weaker emissions in the wavelength range of 500-650 nm, in which the origin was associated with the host matrices. The PL decay curves were approximated by a double exponential decay function for all the Ce-doped samples. The decay times ranged around 10-30 and 40-90 ns, and faster components coincided with those of the non-doped samples. The scintillation decay curves of Ce-doped samples, on the other hand, were approximated by single exponential functions with slower decay constants than those of PL decay. These constants were very similar to those of non-doped samples. In the X-ray induced afterglow measurements, Ce:GCS exhibited the lowest afterglow level. The pulse height spectrum of these samples showed a full-energy peak under 241Am 5.5 MeV α-ray irradiation. Among these samples, Ce:GSrS exhibited the highest light yield which was around 600 ph/5.5 MeV-α.

  17. Divalent fluoride doped cerium fluoride scintillator

    DOEpatents

    Anderson, David F.; Sparrow, Robert W.

    1991-01-01

    The use of divalent fluoride dopants in scintillator materials comprising cerium fluoride is disclosed. The preferred divalent fluoride dopants are calcium fluoride, strontium fluoride, and barium fluoride. The preferred amount of divalent fluoride dopant is less than about two percent by weight of the total scintillator. Cerium fluoride scintillator crystals grown with the addition of a divalent fluoride have exhibited better transmissions and higher light outputs than crystals grown without the addition of such dopants. These scintillators are useful in radiation detection and monitoring applications, and are particularly well suited for high-rate applications such as positron emission tomography (PET).

  18. Crystal structure, electronic structure, temperature-dependent optical and scintillation properties of CsCe2Br7

    SciTech Connect

    Wu, Yuntao; Shi, Hongliang; Chakoumakos, Bryan C.; Zhuravleva, Mariya; Du, Mao-Hua; Melcher, Charles L.

    2015-10-05

    CsCe2Br7 is a self-activated inorganic scintillator that shows promising performance, but the understanding of the important structure-property relationships is lacking. In this work, we conduct a comprehensive study on CCsCe2Br7. The crystal structure of CsCe2Br7 is refined using single crystal X-ray study for the first time. It crystallizes into the orthorhombic crystal system with Pmnb space group. Its electronic structure is revealed by Density Functional Theory (DFT) calculations. Two cerium emission centers are identified and the energy barriers related to the thermal quenching to 4f ground states of Ce3+ for these two Ce centers are evaluated. CsCe2Br7 single crystal has better light yield and energy resolution than CsCe2Cl7, but with an additional slow decay component of 1.7 s. The existence of a deep trap with a depth of 0.9 eV in CsCe2Cl7 contributes to its higher afterglow level in comparison to that of CsCe2Br7. The most possible point defects in CsCe2Cl7 and CsCe2Br7 are proposed by considering the vapour pressure in the growth atmosphere upon melting point.

  19. New Scintillators for Photosensitive Gaseous Detectors

    NASA Astrophysics Data System (ADS)

    Charpak, G.; Peskov, V.; Scigocki, D.; Valbis, J.

    A new family of scintillators are presented. Their properties are similar to those of barium fluoride, and the spectrum of the scintillation emission is between 140 and 300 nm. Our latest efficiency measurements of ethyl ferrocene and triethylamine liquid or caesium iodide solid photocathodes, in parallel-plate avalanche chambers (PPACs) at high electric field, are also presented. We discuss the revolutionary consequences of the combination of the new scintillators with PPACs with semitransparent photocathodes deposited on the crystals, such as high speed, high resistance to radiation damage, compacity, high gamma efficiency, and applications to tracking devices with scintillation optical fibres.

  20. Plastic scintillation dosimetry: Optimal selection of scintillating fibers and scintillators

    SciTech Connect

    Archambault, Louis; Arsenault, Jean; Gingras, Luc; Sam Beddar, A.; Roy, Rene; Beaulieu, Luc

    2005-07-15

    Scintillation dosimetry is a promising avenue for evaluating dose patterns delivered by intensity-modulated radiation therapy plans or for the small fields involved in stereotactic radiosurgery. However, the increase in signal has been the goal for many authors. In this paper, a comparison is made between plastic scintillating fibers and plastic scintillator. The collection of scintillation light was measured experimentally for four commercial models of scintillating fibers (BCF-12, BCF-60, SCSF-78, SCSF-3HF) and two models of plastic scintillators (BC-400, BC-408). The emission spectra of all six scintillators were obtained by using an optical spectrum analyzer and they were compared with theoretical behavior. For scintillation in the blue region, the signal intensity of a singly clad scintillating fiber (BCF-12) was 120% of that of the plastic scintillator (BC-400). For the multiclad fiber (SCSF-78), the signal reached 144% of that of the plastic scintillator. The intensity of the green scintillating fibers was lower than that of the plastic scintillator: 47% for the singly clad fiber (BCF-60) and 77% for the multiclad fiber (SCSF-3HF). The collected light was studied as a function of the scintillator length and radius for a cylindrical probe. We found that symmetric detectors with nearly the same spatial resolution in each direction (2 mm in diameter by 3 mm in length) could be made with a signal equivalent to those of the more commonly used asymmetric scintillators. With augmentation of the signal-to-noise ratio in consideration, this paper presents a series of comparisons that should provide insight into selection of a scintillator type and volume for development of a medical dosimeter.

  1. High resolution scintillation detector with semiconductor readout

    DOEpatents

    Levin, Craig S.; Hoffman, Edward J.

    2000-01-01

    A novel high resolution scintillation detector array for use in radiation imaging such as high resolution Positron Emission Tomography (PET) which comprises one or more parallelepiped crystals with at least one long surface of each crystal being in intimate contact with a semiconductor photodetector such that photons generated within each crystal by gamma radiation passing therethrough is detected by the photodetector paired therewith.

  2. Development of Novel Polycrystalline Ceramic Scintillators

    SciTech Connect

    Wisniewska, Monika; Boatner, Lynn A; Neal, John S; Jellison Jr, Gerald Earle; Ramey, Joanne Oxendine; North, Andrea L; Wisniewski, Monica; Payzant, E Andrew; Howe, Jane Y; Lempicki, Aleksander; Brecher, Charlie; Glodo, J.

    2008-01-01

    For several decades most of the efforts to develop new scintillator materials have concentrated on high-light-yield inorganic single-crystals while polycrystalline ceramic scintillators, since their inception in the early 1980 s, have received relatively little attention. Nevertheless, transparent ceramics offer a promising approach to the fabrication of relatively inexpensive scintillators via a simple mechanical compaction and annealing process that eliminates single-crystal growth. Until recently, commonly accepted concepts restricted the polycrystalline ceramic approach to materials exhibiting a cubic crystal structure. Here, we report our results on the development of two novel ceramic scintillators based on the non-cubic crystalline materials: Lu SiO:Ce (LSO:Ce) and LaBr:Ce. While no evidence for texturing has been found in their ceramic microstructures, our LSO:Ce ceramics exhibit a surprisingly high level of transparency/ translucency and very good scintillation characteristics. The LSO:Ce ceramic scintillation reaches a light yield level of about 86% of that of a good LSO:Ce single crystal, and its decay time is even faster than in single crystals. Research on LaBr:Ce shows that translucent ceramics of the high-light-yield rare-earth halides can also be synthesized. Our LaBr:Ce ceramics have light yields above 42 000 photons/MeV (i.e., 70%of the single-crystal light yield).

  3. Crystal structure and thermal expansion of a CsCe2Cl7 scintillator

    SciTech Connect

    Zhuravleva, M.; Lindsey, A.; Chakoumakos, B. C.; Custelcean, R.; Meilleur, F.; Hughes, R. W.; Kriven, W. M.; Melcher, C. L.

    2015-04-06

    Here we used single-crystal X-ray diffraction data to determine crystal structure of CsCe2Cl7. It crystallizes in a P1121/b space group with a = 19.352(1) Å, b = 19.352(1) Å, c = 14.838(1) Å, γ = 119.87(2) ° , and V = 4818.6(5) Å3. Differential scanning calorimetry measurements combined with the structural evolution of CsCe2Cl7 via X-ray diffractometry over a temperature range from room temperature to the melting point indicates no obvious intermediate solid-solid phase transitions. The anisotropy in the average linear coefficient of thermal expansion of the a axis (21.3 10-6/ °C) with respect to the b and c axes (27.0 10-6/ °C) was determined through lattice parameter refinement of the temperature dependent diffraction patterns. Lastly, these findings suggest that the reported cracking behavior during melt growth of CsCe2Cl7 bulk crystals using conventional Bridgman and Czochralski techniques may be largely attributed to the anisotropy in thermal expansion.

  4. Crystal structure and thermal expansion of a CsCe{sub 2}Cl{sub 7} scintillator

    SciTech Connect

    Zhuravleva, M.; Lindsey, A.; Chakoumakos, B.C.; Custelcean, R.; Meilleur, F.; Hughes, R.W.; Kriven, W.M.; Melcher, C.L.

    2015-07-15

    We used single-crystal X-ray diffraction data to determine crystal structure of CsCe{sub 2}Cl{sub 7}. It crystallizes in a P112{sub 1}/b space group with a=19.352(1) Å, b=19.352(1) Å, c=14.838(1) Å, γ=119.87(2)°, and V=4818.6(5) Å{sup 3}. Differential scanning calorimetry measurements combined with the structural evolution of CsCe{sub 2}Cl{sub 7} via X-ray diffractometry over a temperature range from room temperature to the melting point indicates no obvious intermediate solid–solid phase transitions. The anisotropy in the average linear coefficient of thermal expansion of the a axis (21.3×10{sup –6}/°C) with respect to the b and c axes (27.0×10{sup –6}/°C) was determined through lattice parameter refinement of the temperature dependent diffraction patterns. These findings suggest that the reported cracking behavior during melt growth of CsCe{sub 2}Cl{sub 7} bulk crystals using conventional Bridgman and Czochralski techniques may be largely attributed to the anisotropy in thermal expansion. - Graphical abstract: Three-dimensional quadric surface of thermal expansion coefficient of CsCe{sub 2}Cl{sub 7} at room temperature (sphere – isotropic) and near melting point (ellipsoid – anisotropic). - Highlights: • Crystal structure of CsCe{sub 2}Cl{sub 7} was solved through X-ray diffraction. • Linear coefficients of thermal expansion were determined from in-situ XRD in 25–650 °C. • Anisotropy of the a axis with respect to b and c axes (21.3 vs 27.0×10{sup –6}/°C) was found. • No solid–solid phase transitions were observed via XRD and thermal analysis.

  5. Investigation of double beta decay of {sup 116}Cd with the help of enriched {sup 116}CdWO{sub 4} crystal scintillators

    SciTech Connect

    Polischuk, O. G. Tretyak, V. I.; Barabash, A. S.; Konovalov, S. I.; Umatov, V. I.; Belli, P.; Bernabei, R.; D’Angelo, S.; Cappella, F.; Caracciolo, V.; Cerulli, R.; Laubenstein, M.; Chernyak, D. M.; Danevich, F. A.; Kobychev, V. V.; Mokina, V. M.; Incicchitti, A.; Poda, D. V.; Shlegel, V. N.; Vasiliev, Ya. V.

    2015-10-28

    An experiment to search for 2β processes in {sup 116}Cd with the help of enriched (to 82%) cadmium tungstate crystal scintillators is in progress at the Gran Sasso National Laboratory of the INFN (LNGS, Italy). After 11074 h of data taking in the last configuration, the preliminary estimate for the half-life of 116Cd relatively to 2ν2β decay is T{sub 1/2} = [2.52 ± 0.02(stat.) ± 0.14(syst.)] × 10{sup 19} yr. By using the data of previous stages of the experiment with a similar level of background (≈ 0.1 counts/(keV kg yr) in the energy interval 2.7 – 2.9 MeV; the total time of measurements is 19770 h) we have obtained a new limit on the 0ν2β decay of {sup 116}Cd to the ground state of {sup 116}Sn: T{sub 1/2} ≥ 1.9 × 10{sup 23} yr at 90% C.L. New limits on different 2β processes in {sup 116}Cd (decays with majorons, transitions to the excited levels) are obtained on the level of T{sub 1/2} ≥ 10{sup 20} – 10{sup 22} yr.

  6. Hygroscopicity Evaluation of Halide Scintillators

    SciTech Connect

    Zhuravleva, M; Stand, L; Wei, H; Hobbs, C. L.; Boatner, Lynn A; Ramey, Joanne Oxendine; Burger, Arnold; Rowe, E; Bhattacharya, P.; Tupitsyn, E; Melcher, Charles L

    2014-01-01

    A collaborative study of relative hygroscopicity of anhydrous halide scintillators grown at various laboratories is presented. We have developed a technique to evaluate moisture sensitivity of both raw materials and grown crystals, in which the moisture absorption rate is measured using a gravimetric analysis. Degradation of the scintillation performance was investigated by recording gamma-ray spectra and monitoring the photopeak position, count rate and energy resolution. The accompanying physical degradation of the samples exposed to ambient atmosphere was photographically recorded as well. The results were compared with ben

  7. Cresst-II: dark matter search with scintillating absorbers

    NASA Astrophysics Data System (ADS)

    Angloher, G.; Bucci, C.; Cozzini, C.; von Feilitzsch, F.; Frank, T.; Hauff, D.; Henry, S.; Jagemann, Th.; Jochum, J.; Kraus, H.; Majorovits, B.; Ninkovic, J.; Petricca, F.; Pröbst, F.; Ramachers, Y.; Rau, W.; Seidel, W.; Stark, M.; Uchaikin, S.; Stodolsky, L.; Wulandari, H.

    2004-03-01

    In the CRESST-II experiment, scintillating CaWO4 crystals are used as absorbers for direct weakly interacting massive particles (WIMP) detection. Nuclear recoils can be discriminated against electron recoils by measuring phonons and scintillation light simultaneously. The absorber crystal and the silicon light detector are read out by tungsten superconducting phase transition thermometers. Results on the sensitivity of the phonon and the light channel, radiopurity, the scintillation properties of CaWO4, and on the WIMP sensitivity are presented.

  8. Characterization of the scintillation anisotropy in crystalline stilbene scintillator detectors

    SciTech Connect

    Schuster, P.; Brubaker, E.

    2016-11-23

    This study reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline melt-grown and solution-grown trans-stilbene to incident DT and DD neutrons. These measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature for melt-grown stilbene and providing the first measurements for solution-grown stilbene. In similar measurements of liquid and plastic detectors, no directional dependence was observed, confirming the hypothesis that the anisotropy in stilbene and other organic crystal scintillators is a result of internal effects due to the molecular or crystal structure and not an external effect on the measurement system.

  9. Characterization of the scintillation anisotropy in crystalline stilbene scintillator detectors

    DOE PAGES

    Schuster, P.; Brubaker, E.

    2016-11-23

    This study reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline melt-grown and solution-grown trans-stilbene to incident DT and DD neutrons. These measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature for melt-grown stilbene and providing the first measurements for solution-grown stilbene. In similar measurements of liquid and plastic detectors, no directional dependence was observed, confirming the hypothesis that the anisotropy in stilbene and other organic crystal scintillators is a result of internal effects duemore » to the molecular or crystal structure and not an external effect on the measurement system.« less

  10. Non-Carbon Dyes For Platic Scintillators- Report

    SciTech Connect

    Teprovich, J.; Colon-Mercado, H.; Gaillard, J.; Sexton, L.; Washington, A.; Ward, P.; Velten, J.

    2015-10-19

    Scintillation based detectors are desirable for many radiation detection applications (portal and border monitoring, safeguards verification, contamination detection and monitoring). The development of next generation scintillators will require improved detection sensitivity for weak gamma ray sources, and fast and thermal neutron quantification. Radiation detection of gamma and neutron sources can be accomplished with organic scintillators, however, the single crystals are difficult to grow for large area detectors and subject to cracking. Alternatives to single crystal organic scintillators are plastic scintillators (PS) which offer the ability to be shaped and scaled up to produce large sized detectors. PS is also more robust than the typical organic scintillator and are ideally suited for deployment in harsh real-world environments. PS contain a mixture of dyes to down-convert incident radiation into visible light that can be detected by a PMT. This project will evaluate the potential use of nano-carbon dyes in plastic scintillators.

  11. Estimation of Fano factor in inorganic scintillators

    PubMed Central

    Bora, Vaibhav; Barrett, Harrison H.; Fastje, David; Clarkson, Eric; Furenlid, Lars; Bousselham, Abdelkader; Shah, Kanai S.; Glodo, Jarek

    2015-01-01

    The Fano factor of an integer-valued random variable is defined as the ratio of its variance to its mean. Correlation between the outputs of two photomultiplier tubes on opposite faces of a scintillation crystal was used to estimate the Fano factor of photoelectrons and scintillation photons. Correlations between the integrals of the detector outputs were used to estimate the photoelectron and photon Fano factor for YAP:Ce, SrI2:Eu and CsI:Na scintillator crystals. At 662 keV, SrI2:Eu was found to be sub-Poisson, while CsI:Na and YAP:Ce were found to be super-Poisson. An experiment setup inspired from the Hanbury Brown and Twiss experiment was used to measure the correlations as a function of time between the outputs of two photomultiplier tubes looking at the same scintillation event. A model of the scintillation and the detection processes was used to generate simulated detector outputs as a function of time for different values of Fano factor. The simulated outputs from the model for different Fano factors was compared to the experimentally measured detector outputs to estimate the Fano factor of the scintillation photons for YAP:Ce, LaBr3:Ce scintillator crystals. At 662 keV, LaBr3:Ce was found to be sub-Poisson, while YAP:Ce was found to be close to Poisson. PMID:26644631

  12. Fracture-resistant lanthanide scintillators

    DOEpatents

    Doty, F. Patrick

    2011-01-04

    Lanthanide halide alloys have recently enabled scintillating gamma ray spectrometers comparable to room temperature semiconductors (<3% FWHM energy resolutions at 662 keV). However brittle fracture of these materials upon cooling hinders the growth of large volume crystals. Efforts to improve the strength through non-lanthanide alloy substitution, while preserving scintillation, have been demonstrated. Isovalent alloys having nominal compositions of comprising Al, Ga, Sc, Y, and In dopants as well as aliovalent alloys comprising Ca, Sr, Zr, Hf, Zn, and Pb dopants were prepared. All of these alloys exhibit bright fluorescence under UV excitation, with varying shifts in the spectral peaks and intensities relative to pure CeBr.sub.3. Further, these alloys scintillate when coupled to a photomultiplier tube (PMT) and exposed to .sup.137Cs gamma rays.

  13. Energy resolution measurements of LaBr 3:Ce scintillating crystals with an ultra-high quantum efficiency photomultiplier tube

    NASA Astrophysics Data System (ADS)

    Pani, R.; Cinti, M. N.; Scafè, R.; Pellegrini, R.; Vittorini, F.; Bennati, P.; Ridolfi, S.; Lo Meo, S.; Mattioli, M.; Baldazzi, G.; Pisacane, F.; Navarria, F.; Moschini, G.; Boccaccio, P.; Orsolini Cencelli, V.; Sacco, D.

    2009-10-01

    The performance of the new prototype of high quantum efficiency PMT (43% at 380 nm), Hamamatsu R7600U-200, was studied coupled to a LaBr 3:Ce crystal with the size of ∅12.5 mm×12.5 mm. The energy resolution results were compared with ones from two PMTs, Hamamatsu R7600U and R6231MOD, with 22% and 30% quantum efficiency (QE), respectively. Moreover, the photodetectors were equipped with tapered and un-tapered voltage dividers to study the non-linearity effects on pulse height distribution, due to very high peak currents induced in the PMT by the fast and intense light pulse of LaBr 3:Ce. The results show an energy resolution improvement with UBA PMT of about 20%, in the energy range of 80-662 keV, with respect to the BA one.

  14. Multilayer passive shielding of scintillation detectors based on BGO, NaI(Tl), and stilbene crystals operating in intense neutron fields with an energy of 14.1 MeV

    NASA Astrophysics Data System (ADS)

    Bystritsky, V. M.; Valkovic, V.; Grozdanov, D. N.; Zontikov, A. O.; Ivanov, I. Zh.; Kopatch, Yu. N.; Krylov, A. R.; Rogov, Yu. N.; Ruskov, I. N.; Sapozhnikov, M. G.; Skoy, V. R.; Shvetsov, V. N.

    2015-03-01

    We discuss the issues related to choosing the optimum type of passive shielding of scintillation detectors based on BGO, NaI(Tl), and stilbene crystals from the direct penetration of neutron radiation with an energy of 14.1 MeV that was emitted isotropically into a solid angle of 4π. A series of experimental measurements of the count-rate suppression factor that may be obtained for the indicated detectors through the use of various shielding filters comprising iron, lead, and borated polyethylene layers with a total thickness not exceeding 50 cm are conducted.

  15. Energy Transfer Based Nanocomposite Scintillator for Radiation Detection

    NASA Astrophysics Data System (ADS)

    Aslam, Soha; Sahi, Sunil; Chen, Wei; Ma, Lun; Kenarangui, Rasool

    2014-09-01

    Scintillators are the materials that emit light upon irradiation with high energy radiation like X-ray or gamma-ray. Inorganic single crystal and organic (plastic and liquid) are the two most used scintillator types. Both of these scintillator kinds have advantages and disadvantages. Inorganic single crystals are expensive and difficult to grow in desire shape and size. Also, single crystal scintillator such as NaI and CsI are very hygroscopic. On the other hand, organic scintillators have low density which limits their applications in gamma spectroscopy. Due to high quantum yield and size dependent emission, nanoparticles have attracted interested in various field of research. Here, we have studies the nanoparticles for radiation detection. We have synthesized nanoparticles of Cerium fluoride (CeF3), Zinc Oxide (ZnO), Cadmium Telluride (CdTe), Copper complex and Zinc sulfide (ZnS). We have used Fluorescence Resonance Energy Transfer (FRET) principle to enhance the luminescence properties of nanocomposite scintillator. Nanocomposites scintillators are structurally characterized with X-ray diffraction (XRD) and Transmission Electron Microscopy (TEM). Optical properties are studied using Photoluminescence, UV-Visible and X-ray. Enhancements in the luminescence are observed under UV and X-ray excitation. Preliminary studies shows nanocomposite scintillators are promising for radiation detection. Scintillators are the materials that emit light upon irradiation with high energy radiation like X-ray or gamma-ray. Inorganic single crystal and organic (plastic and liquid) are the two most used scintillator types. Both of these scintillator kinds have advantages and disadvantages. Inorganic single crystals are expensive and difficult to grow in desire shape and size. Also, single crystal scintillator such as NaI and CsI are very hygroscopic. On the other hand, organic scintillators have low density which limits their applications in gamma spectroscopy. Due to high quantum

  16. Optical transmission radiation damage and recovery stimulation of DSB: Ce3+ inorganic scintillation material

    NASA Astrophysics Data System (ADS)

    Borisevich, A.; Dormenev, V.; Korjik, M.; Kozlov, D.; Mechinsky, V.; Novotny, R. W.

    2015-02-01

    Recently, a new scintillation material DSB: Ce3+ was announced. It can be produced in a form of glass or nano-structured glass ceramics with application of standard glass production technology with successive thermal annealing. When doped with Ce3+, material can be applied as scintillator. Light yield of scintillation is near 100 phe/MeV. Un-doped material has a wide optical window from 4.5eV and can be applied to detect Cherenkov light. Temperature dependence of the light yield LY(T) is 0.05% which is 40 times less than in case of PWO. It can be used for detectors tolerant to a temperature variation between -20° to +20°C. Several samples with dimensions of 15x15x7 mm3 have been tested for damage effects on the optical transmission under irradiation with γ-quanta. It was found that the induced absorption in the scintillation range depends on the doping concentration and varies in range of 0.5-7 m-1. Spontaneous recovery of induced absorption has fast initial component. Up to 25% of the damaged transmission is recuperated in 6 hours. Afterwards it remains practically constant if the samples are kept in the dark. However, induced absorption is reduced by a factor of 2 by annealing at 50°C and completely removed in a short time when annealing at 100°C. A significant acceleration of the induced absorption recovery is observed by illumination with visible and IR light. This effect is observed for the first time in a Ce-doped scintillation material. It indicates, that radiation induced absorption in DSB: Ce scintillation material can be retained at the acceptable level by stimulation with light in a strong irradiation environment of collider experiments.

  17. Scintillators and applications thereof

    DOEpatents

    Williams, Richard T.

    2015-09-01

    Scintillators of various constructions and methods of making and using the same are provided. In some embodiments, a scintillator comprises at least one radiation absorption region and at least one spatially discrete radiative exciton recombination region.

  18. Scintillators and applications thereof

    DOEpatents

    Williams, Richard T.

    2014-07-15

    Scintillators of various constructions and methods of making and using the same are provided. In some embodiments, a scintillator comprises at least one radiation absorption region and at least one spatially discrete radiative exciton recombination region.

  19. Scintillator manufacture at Fermilab

    SciTech Connect

    Mellott, K.; Bross, A.; Pla-Dalmau, A.

    1998-08-01

    A decade of research into plastic scintillation materials at Fermilab is reviewed. Early work with plastic optical fiber fabrication is revisited and recent experiments with large-scale commercial methods for production of bulk scintillator are discussed. Costs for various forms of scintillator are examined and new development goals including cost reduction methods and quality improvement techniques are suggested.

  20. Lead carbonate scintillator materials

    DOEpatents

    Derenzo, Stephen E.; Moses, William W.

    1991-01-01

    Improved radiation detectors containing lead carbonate or basic lead carbonate as the scintillator element are disclosed. Both of these scintillators have been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to other known scintillator materials. The radiation detectors disclosed are favorably suited for use in general purpose detection and in medical uses.

  1. Scintillation properties of polycrystalline LaxY1-xO3 ceramic

    NASA Astrophysics Data System (ADS)

    Sahi, Sunil; Chen, Wei; Kenarangui, Rasool

    2015-03-01

    Scintillators are the material that absorbs the high-energy photons and emits visible photons. Scintillators are commonly used in radiation detector for security, medical imaging, industrial applications and high energy physics research. Two main types of scintillators are inorganic single crystals and organic (plastic or liquid) scintillators. Inorganic single crystals are expensive and difficult to grow in desire shape and size. Also, some efficient inorganic scintillator such as NaI and CsI are not environmental friendly. But on the other hand, organic scintillators have low density and hence poor energy resolution which limits their use in gamma spectroscopy. Polycrystalline ceramic can be a cost effective alternative to expensive inorganic single crystal scintillators. Here we have fabricated La0.2Y1.8O3 ceramic scintillator and studied their luminescence and scintillation properties. Ceramic scintillators were fabricated by vacuum sintering of La0.2Y1.8O3 nanoparticles at temperature below the melting point. La0.2Y1.8O3 ceramic were characterized structurally using XRD and TEM. Photoluminescence and radioluminescence studies were done using UV and X-ray as an excitation source. We have used gamma isotopes with different energy to studies the scintillation properties of La0.2Y1.8O3 scintillator. Preliminary studies of La0.2Y1.8O3 scintillator shows promising result with energy resolution comparable to that of NaI and CsI.

  2. Scintillator reflective layer coextrusion

    DOEpatents

    Yun, Jae-Chul; Para, Adam

    2001-01-01

    A polymeric scintillator has a reflective layer adhered to the exterior surface thereof. The reflective layer comprises a reflective pigment and an adhesive binder. The adhesive binder includes polymeric material from which the scintillator is formed. A method of forming the polymeric scintillator having a reflective layer adhered to the exterior surface thereof is also provided. The method includes the steps of (a) extruding an inner core member from a first amount of polymeric scintillator material, and (b) coextruding an outer reflective layer on the exterior surface of the inner core member. The outer reflective layer comprises a reflective pigment and a second amount of the polymeric scintillator material.

  3. Design studies of the PWO Forward End-cap calorimeter for P¯ANDA

    NASA Astrophysics Data System (ADS)

    Moeini, H.; Al-Turany, M.; Babai, M.; Biegun, A.; Bondarenko, O.; Götzen, K.; Kavatsyuk, M.; Lindemulder, M. F.; Löhner, H.; Melnychuk, D.; Messchendorp, J. G.; Smit, H. A. J.; Spataro, S.; Veenstra, R.

    2013-11-01

    The P¯ANDA detection system at FAIR, Germany, is designed to study antiproton-proton annihilations, in order to investigate, among others, the realm of charm-meson states and glueballs, which has still much to reveal. The yet unknown properties of this field are to be unraveled through studying QCD phenomena in the non-perturbative regime. The multipurpose P¯ANDA detector will be capable of tracking, calorimetry, and particle identification, and is planned to run at high luminosities providing average reaction rates up to 2 · 107 interactions/s. The envisaged physics program requires measurements of photons and charged particles with excellent energy, position, and time resolutions. The electromagnetic calorimeter (EMC) will serve as one of the basic components of the detector setup and comprises cooled lead-tungstate (PbWO4) crystals. This paper presents the mechanical design of the Forward End-cap calorimeter and analyzes the response of the Forward End-cap calorimeter in conjunction with the full EMC and the complete P¯ANDA detector. The simulation studies are focused on the performance of the planned EMC with respect to the energy and spatial resolution of the reconstructed photons. Results of the Monte Carlo simulations, excluding very low-energy photons, have been validated by data obtained from a prototype calorimeter and shown to fulfil the requirements imposed by the P¯ANDA physics program.

  4. Elpasolite scintillators.

    SciTech Connect

    Doty, F. Patrick; Zhou, Xiao Wang; Yang, Pin; Rodriguez, Mark A

    2012-12-01

    This work was funded by the U.S. Department of Energy Office of Nonproliferation Research to develop elpasolite materials, with an emphasis on high-atomic-number rare-earth elpasolites for gamma-ray spectrometer applications. Low-cost, high-performance gamma-ray spectrometers are needed for detection of nuclear proliferation. Cubic materials, such as some members of the elpasolite family (A2BLnX6; Ln-lanthanide and X-halogen), hold promise due to their high light output, proportionality, and potential for scale-up. Using both computational and experimental studies, a systematic investigation of the compositionstructureproperty relationships of these high-atomic-number elpasolite halides was performed. The results reduce the barrier to commercialization of large single crystals or transparent ceramics, and will facilitate economical scale-up of elpasolites for high-sensitivity gamma-ray spectroscopy.

  5. Shifting scintillator neutron detector

    DOEpatents

    Clonts, Lloyd G; Cooper, Ronald G; Crow, Jr., Morris Lowell; Hannah, Bruce W; Hodges, Jason P; Richards, John D; Riedel, Richard A

    2014-03-04

    Provided are sensors and methods for detecting thermal neutrons. Provided is an apparatus having a scintillator for absorbing a neutron, the scintillator having a back side for discharging a scintillation light of a first wavelength in response to the absorbed neutron, an array of wavelength-shifting fibers proximate to the back side of the scintillator for shifting the scintillation light of the first wavelength to light of a second wavelength, the wavelength-shifting fibers being disposed in a two-dimensional pattern and defining a plurality of scattering plane pixels where the wavelength-shifting fibers overlap, a plurality of photomultiplier tubes, in coded optical communication with the wavelength-shifting fibers, for converting the light of the second wavelength to an electronic signal, and a processor for processing the electronic signal to identify one of the plurality of scattering plane pixels as indicative of a position within the scintillator where the neutron was absorbed.

  6. CRESST-II: dark matter search with scintillating absorbers

    NASA Astrophysics Data System (ADS)

    Angloher, G.; Bucci, C.; Cozzini, C.; von Feilitzsch, F.; Frank, T.; Hauff, D.; Henry, S.; Jagemann, Th.; Jochum, J.; Kraus, H.; Majorovits, B.; Ninkovic, J.; Petricca, F.; Pröbst, F.; Ramachers, Y.; Rau, W.; Seidel, W.; Stark, M.; Uchaikin, S.; Stodolsky, L.; Wulandari, H.

    2005-01-01

    In the CRESST-II experiment, scintillating CaWO 4 crystals are used as absorbers for direct WIMP (weakly interacting massive particles) detection. Nuclear recoils can be discriminated against electron recoils by measuring phonons and scintillation light simultaneously. The absorber crystal and the silicon light detector are read out by tungsten superconducting phase transition thermometers (W-SPTs). Results on the sensitivity of the phonon and the light channel, radiopurity, the scintillation properties of CaWO 4, and on the WIMP sensitivity are presented.

  7. Study of equatorial scintillations

    NASA Technical Reports Server (NTRS)

    Pomalaza, J.; Woodman, R.; Tisnado, G.; Nakasone, E.

    1972-01-01

    Observations of the amplitude scintillations produced by the F-region in equatorial areas are presented. The equipment used for conducting the observations is described. The use of transmissions from the ATS-1, ATS-3, and ATS-5 for obtaining data is described. The two principal subjects discussed are: (1) correlation between satellite and incoherent radar observations of scintillations and (2) simultaneous observations of scintillations at 136 MHz and 1550 MHz.

  8. Lead carbonate scintillator materials

    DOEpatents

    Derenzo, S.E.; Moses, W.W.

    1991-05-14

    Improved radiation detectors containing lead carbonate or basic lead carbonate as the scintillator element are disclosed. Both of these scintillators have been found to provide a balance of good stopping power, high light yield and short decay constant that is superior to other known scintillator materials. The radiation detectors disclosed are favorably suited for use in general purpose detection and in medical uses. 3 figures.

  9. Accelerated discovery of elpasolite scintillators

    SciTech Connect

    Doty, F. Patrick; Yang, Pin; Zhou, Xiaowang

    2014-12-01

    Elpasolite scintillators are a large family of halides which includes compounds reported to meet the NA22 program goals of <3% energy resolution at 662 keV1. This work investigated the potential to produce quality elpasolite compounds and alloys of useful sizes at reasonable cost, through systematic experimental and computational investigation of crystal structure and properties across the composition space. Discovery was accelerated by computational methods and models developed previously to efficiently identify cubic members of the elpasolite halides, and to evaluate stability of anion and cation exchange alloys.

  10. Purification of large liquid scintillators for Borexino

    SciTech Connect

    Benziger, J.B.; Calaprice, F.P.; Vogelaar, R.B.

    1993-10-01

    Distillation extraction and crystallization have been used on scintillator mixtures for solar neutrino physics to remove cosmo- genically produced impurities ({sup 7}Be) and naturally occurring impurities ({sup 238}U, {sup 232}Th, and {sup 40}K), and to improve the optical transmission. Distillation was effective at removing {sup 7}Be and other impurities from aromatic solvents (p-xylene and pseudocumene) used as scintillator solvents. Distillation also provided the greatest improvement in the optical clarity of the solvents. Commercially available fluors (PPO and PMP) have high levels of potassium, far in excess of those tolerable for Borexino. Extraction techniques have been found to be effective at removing radioactive impurities, particularly potassium, from the fluors. An overall strategy for on-line purification of the scintillator for Borexino will be presented.

  11. Development of a novel depth-of-interaction encoding method and use of light spreading in a scintillation crystal array with single-ended readout

    NASA Astrophysics Data System (ADS)

    Lee, Seung-Jae; Lee, Chaeyeong; Chung, Yong Hyun; Kang, Jihoon; Baek, Cheol-Ha

    2016-12-01

    We designed a depth-of-interaction (DOI) positron emission tomography detector by applying a simple light-spreading method in a single-layer crystal array with a single-ended photosensor. By configuring different reflector patterns along the depth of the crystal, we were able to alter the light distribution of the gamma interaction at each depth. To evaluate the characteristics of the new DOI detector, we simulated the optical photon transport in the crystal array by using DETECT2000. Three different arrays comprising triangular-, square-, and hexagonal-shaped crystals were modeled. The 511-keV gamma-ray interactions were generated for all depths, and flood images were acquired. We confirmed that DOI layers could be distinguished in the obtained images and that the number of DOI layers depends on the number of sides of the polygonal crystals.

  12. Mercuric iodide photodetectors for scintillation spectroscopy

    SciTech Connect

    Markakis, J.; Dabrowski, A.; Iwanczyk, J.; Ortale, C.; Schnepple, W.

    1985-02-01

    We have measured the responses to /sup 137/Cs (662 keV) of both a 1-inch-diam by 2-inch-thick NaI(Tl) scintillator optically coupled to a 1-inch-diam by 800-..mu..mthick mercuric iodide (HgI/sub 2/) photodetector, and a 1-cmdiam by 1-cm-thick CaWO/sub 4/ scintillator coupled to a 1.3-cm-diam by 600-..mu..m-thick HgI/sub 2/ photodetector. Best spectral resolution to /sup 137/Cs was 7.8% FWHM for the NaI(Tl)-HgI/sub 2/ and 12.5% FWHM for the CaWO/sub 4/-HgI/sub 2/ detectors; peak-to-valley ratios were 26:1 and 16:1, respectively. HgI/sub 2/ detectors operate at room temperature and their use in scintillation spectroscopy presents the ultimate miniaturization of scintillation detectors, limited mainly by the size of the scintillation crystal.

  13. Mercuric iodide photodetectors for scintillation spectroscopy

    SciTech Connect

    Markakis, J.; Ortale, C.; Schnepple, W.; Iwanczyk, J.; Dabrowski, A.

    1984-01-01

    We have measured the responses to /sup 137/Cs (662 keV) of both a 1-inch-diam by 2-inch-thick NaI(Tl) scintillator optically coupled to a 1-inch-diam by 800-..mu..m-thick mercuric iodide (HgI/sub 2/) photodetector, and a 1-cm-diam by 1-cm-thick CaWO/sub 4/ scintillator coupled to a 1.3-cm-diam by 600-..mu..m-thick HgI/sub 2/ photodetector. Best spectral resolution to /sup 137/Cs was 7.8% FWHM for the NaI(Tl)-HgI/sub 2/ and 12.5% FWHM for the CaWO/sub 4/-HgI/sub 2/ detectors; peak-to-valley ratios were 26:1 and 16:1, respectively. HgI/sub 2/ detectors operate at room temperature and their use in scintillation spectroscopy presents the ultimate miniaturization of scintillation detectors, limited mainly by the size of the scintillation crystal.

  14. Luminescence quenching and scintillation response in the Ce3+ doped GdxY3-xAl5O12 (x = 0.75, 1, 1.25, 1.5, 1.75, 2) single crystals

    NASA Astrophysics Data System (ADS)

    Bartosiewicz, K.; Babin, V.; Kamada, K.; Yoshikawa, A.; Mares, J. A.; Beitlerova, A.; Nikl, M.

    2017-01-01

    The luminescence and scintillation properties of the gadolinium yttrium aluminium garnets, (Gd,Y)3Al5O12 doped with Ce3+ are investigated as a function of the Gd/Y ratio with the aim of an improved understanding of the luminescence quenching, energy transfer and phase stability in these materials. An increase of both crystal field strength and instability of the garnet phase with increasing content of Gd3+ is observed. The instability of the garnet phase results in an appearance of the perovskite phase inclusions incorporated into the garnet phase. The luminescence features of Ce3+ in the perovskite phase inclusions and in the main garnet phase are studied separately. The thermal quenching of the 5 d → 4f emission of Ce3+ in the latter phase is determined by temperature dependence of the photoluminescence decay time. The results show that the onset of the thermal quenching is moved to lower temperatures with increasing gadolinium content. The measurements of temperature dependence of delayed radiative recombination do not reveal a clear evidence that the thermal quenching is caused by thermally induced ionization of the Ce3+ 5d1 excited state. Therefore, the main mechanism responsible for the luminescence quenching is due to the non-radiative relaxation from 5d1 excited state to 4f ground state of Ce3+. The energy transfer processes between Gd3+ and Ce3+ as well as between perovskite and garnet phases are evidenced by the photoluminescence excitation and emission spectra as well as decay kinetic measurements. Thermally stimulated luminescence (TSL) studies in the temperature range 77-497 K and scintillation decays under γ excitation complete the material characterization.

  15. THE CRYSTAL STRUCTURE OF 2,7-DIACETOXYTRANS-15,16-DIMETHYL-15,16-DIHYDROPYRENE,

    DTIC Science & Technology

    AROMATIC COMPOUNDS, CRYSTAL STRUCTURE ), (*POLYCYCLIC COMPOUNDS, CRYSTAL STRUCTURE ), (* CRYSTAL STRUCTURE , POLYCYCLIC COMPOUNDS), ESTERS, MOLECULAR STRUCTURE, CHEMICAL BONDS, X RAY DIFFRACTION, SCINTILLATION COUNTERS, CANADA

  16. Simulation of scintillation light output in LYSO scintillators through a full factorial design

    NASA Astrophysics Data System (ADS)

    Loignon-Houle, Francis; Bergeron, Mélanie; Pepin, Catherine M.; Charlebois, Serge A.; Lecomte, Roger

    2017-01-01

    Individually coupled scintillation detectors used in positron emission tomography (PET) imaging suffer from important signal losses due to the suboptimal light collection from crystals. As only a fraction of the light is generally extracted from long and thin scintillators, it is important to identify and understand the predominant causes of signal loss in order to eventually recover it. This simulation study investigates the multiple factors affecting the light transport in high-aspect ratio LYSO scintillators wrapped in specular reflectors through a full factorial design. By exploring various combinations of crystal geometry, readout conditions and wrapping conditions, it was found that an optimum light output can only be achieved through a careful selection of highly reflective material along with high-transmittance optical adhesive used to bond the reflector. Decreasing the adhesive thickness was also found to have a positive outcome in most explored configurations, however to a much lesser extent. Suboptimal reflectivity and adhesive transmittance also lead to an asymmetric light output distribution dependent on the depth of interaction of the radiation, potentially degrading energy resolution. By identifying the factors causing the most significant scintillation light losses through a factorial design, the most promising detector configurations have been identified in the quest for optimal light collection from scintillators.

  17. A comparative study of gamma-ray spectrometers with LaBr3(Ce3+) and CeBr3 scintillation crystals for planetary remote sensing applications.

    NASA Astrophysics Data System (ADS)

    Kozyrev, Alexander; Mitrofanov, Igor; Owens, Alan; Quarati, Francesco; Benkhoff, Johannes; Litvak, Maxim; Malakhov, Alexey; Mokrousov, Maxim; Vostrukhin, Andrey; Golovin, Dmitry; Tretyakov, Vladislav; Sanin, Anton; Bakhtin, Boris; Timoshenko, Gennady; Shvetsov, Valery; Granja, Carlos; Slavicek, Tomáš; Pospisil, Stanislav

    2016-04-01

    The Russian Space Research Institute has developed and manufactured the gamma-ray spectrometer MGNS for remote sensing observations of the Mercury from the Mercury Polar Orbiter (MPO), which is the part of ESA's BepiColombo mission. The Flight Model (FM) of MGNS is based on a 3-inch single crystal of LaBr3(Ce3+), which was produced in the crystal development programme specifically for this mission. During the instrument development and verification, the crystals of CeBr3(Ce3+) became available with the similar sizes in a subsequent phase of the same crystal development programme. Consequently, the Flight Spare Model (FSM) of MGNS was produced with the 3-inch CeBr3 crystal and qualified for space flight. Except for the crystals, the two units FM and FSM are essentially identical. We report the results on a comparative assessment of the two units in terms of their respective spectroscopic capabilities, well as for their suitability for interplanetary spacecraft with respect to radiation tolerance and redundancy for activation. We also compare their performance with that of the Ge detector, as one used on the Messenger mission. Based on the tests results, the decision was taken to use FSM onboard the MPO on the BepiColombo mission. Thus, the MGNS with CeBr3 is the central gamma-ray detection element on the MPO spacecraft.

  18. YAP:Ce scintillator characteristics for neutron detection

    SciTech Connect

    Viererbl, L.; Klupak, V.; Vins, M.; Soltes, J.

    2015-07-01

    YAP:Ce (YAlO{sub 3}:Ce{sup +}, Yttrium Aluminum Perovskite, Ce{sup +} doped) crystals with appropriate converters seem like prospective scintillators for neutron detection. An important aspect for neutron detection with inorganic scintillators is the ability to discriminate neutron radiation from gamma radiation by pulse height of signals. For a detailed measurement of the aspect, a YAP:Ce crystal scintillator with lithium or hydrogen converters and a photomultiplier was used. A plutonium-beryllium neutron source and horizontal neutron channel beams of the LVR-15 research reactor were used as neutron sources. The measurement confirmed the possibility to use the YAP:Ce scintillator for neutron radiation detection. The degree of discrimination between neutron and gamma radiation for different detection configurations was studied. (authors)

  19. Development of scintillation materials for medical imaging and other applications

    SciTech Connect

    Melcher, C. L.

    2013-02-05

    Scintillation materials that produce pulses of visible light in response to the absorption of energetic photons, neutrons, and charged particles, are widely used in various applications that require the detection of radiation. The discovery and development of new scintillators has accelerated in recent years, due in large part to their importance in medical imaging as well as in security and high energy physics applications. Better understanding of fundamental scintillation mechanisms as well as the roles played by defects and impurities have aided the development of new high performance scintillators for both gamma-ray and neutron detection. Although single crystals continue to dominate gamma-ray based imaging techniques, composite materials and transparent optical ceramics potentially offer advantages in terms of both synthesis processes and scintillation performance. A number of promising scintillator candidates have been identified during the last few years, and several are currently being actively developed for commercial production. Purification and control of raw materials and cost effective crystal growth processes can present significant challenges to the development of practical new scintillation materials.

  20. Influence of Depth of Interaction upon the Performance of Scintillator Detectors

    PubMed Central

    Brown, Mark S.; Gundacker, Stefan; Taylor, Alaric; Tummeltshammer, Clemens; Auffray, Etiennette; Lecoq, Paul; Papakonstantinou, Ioannis

    2014-01-01

    The uncertainty in time of particle detection within a scintillator detector, characterised by the coinci- dence time resolution (CTR), is explored with respect to the interaction position within the scintillator crystal itself. Electronic collimation between two scintillator detectors is utilised to determine the CTR with depth of interaction (DOI) for different materials, geometries and wrappings. Significantly, no rela- tionship between the CTR and DOI is observed within experimental error. Confinement of the interaction position is seen to degrade the CTR in long scintillator crystals by 10%. PMID:24875832

  1. Scintillating pad detectors

    SciTech Connect

    Adams, D.; Baumbaugh, B.; Borcherding, F.

    1996-12-31

    We have been investigating the performance of scintillating pad detectors, individual small tiles of scintillator that are read out with wavelength-shifting fibers and visible light photon counters, for application in high luminosity colliding beam experiments such as the D0 Upgrade. Such structures could provide {open_quotes}pixel{close_quotes} type readout over large fiducial volumes for tracking, preshower detection and triggering.

  2. Co-doping effects on luminescence and scintillation properties of Ce doped (Lu,Gd)3(Ga,Al)5O12 scintillator

    NASA Astrophysics Data System (ADS)

    Yamaguchi, Hiroaki; Kamada, Kei; Kurosawa, Shunsuke; Pejchal, Jan; Shoji, Yasuhiro; Yokota, Yuui; Ohashi, Yuji; Yoshikawa, Akira

    2016-11-01

    Mg co-doping effects on scintillation properties of Ce:Lu1Gd2(Ga,Al)5O12 (LGGAG) were investigated. Mg 200 ppm co-doped Ce:LGGAG single crystals were prepared by micro pulling down method. Absorption and luminescence spectra were measured together with several other scintillation characteristics, namely the scintillation decay and light yield to reveal the effect of Mg co-doping. Ce4+ charge transfer absorption was observed below 300 nm in Mg,Ce:LGGAG which is in good agreement with previous reports. The scintillation decay times were accelerated by Mg co-doping.

  3. Application of the Scintillation Detector on base of BrilLanCe Series Crystal in Neutral Particles Spectrometer for the Satellite Experiment ZINA-NT

    NASA Astrophysics Data System (ADS)

    Arkhangelskaja, Irene; Arkhangelsky, Andrey; Batischev, Alexey; Naumov, Pietr; Kondratyeva, Natalia

    In a condition of normal gravity, field-induced translational and rotational motions of solids are publically recognized for materials that contain spontaneous magnetic moments. It is believed that a high field above B = 10 T is necessary to induce such movements for ordinary diamagnetic material. Rotation and translation induced by low field of B = 0.5 T were recently reported on diamagnetic single-crystals of corundum [1], calcite, diamond, graphite and silver [2]. Here the crystals were released in microgravity produced by drop capsule(duration 4.5 s), and the motions took place in diffused gas medium (50Pa). In homogeneous field, crystal showed rotational oscillation with respect to field because of diamagnetic anisotropy energy. In a given field intensity, its period was determined by anisotropy of diamagnetic susceptibility. The crystal was ejected from field center by field-gradient force with significant terminal velocity. In a given field distribution, the velocity uniquely depended on intrinsic susceptibility of material. It is expected that the above two motions were independent to mass of sample. Necessity of clarifying magnetic properties of a single particle is increasing with the growing interest on nano-sized materials; data of susceptibility as well as its anisotropy are necessary for characterizing its property. However the values are difficult to obtain by conventional methods because of 2 factors; existence of a sample holder, and necessity of mass measurement. Susceptibility and its anisotropy of a single particle can be determined with high precision from above two motions in microgravity, because the methods are free of sample holder and mass measurement. Moreover, they are based on simple motional equations that consist of an inertia term and a magnetic term. In principle, magnetization is measured for limitlessly small sample, provided that the motions are observed. Attempt to obtain magnetization curve from the above-mentioned translation

  4. Scintillator Measurements for SNO+

    NASA Astrophysics Data System (ADS)

    Kaptanoglu, Tanner; SNO+ Collaboration

    2016-03-01

    SNO+ is a neutrino detector located 2km underground in the SNOLAB facility with the primary goal of searching for neutrinoless double beta decay. The detector will be filled with a liquid scintillator target primarily composed of linear alkyl benzene (LAB). As charged particles travel through the detector the LAB produces scintillation light which is detected by almost ten thousand PMTs. The LAB is loaded with Te130, an isotope known to undergo double beta decay. Additionally, the LAB is mixed with an additional fluor and wavelength shifter to improve the light output and shift the light to a wavelength regime in which the PMTs are maximally efficient. The precise scintillator optics drastically affect the ultimate sensitivity of SNO+. I will present work being done to measure the optical properties of the SNO+ scintillator cocktail. The measured properties are used as input to a scintillation model that allows us to extrapolate to the SNO+ scale and ultimately predict the sensitivity of the experiment. Additionally, I will present measurements done to characterize the R5912 PMT, a candidate PMT for the second phase of SNO+ that provides better light collection, improved charge resolution, and a narrower spread in timing.

  5. Evaluate Scintillation Response Over a Continuous Energy Region

    SciTech Connect

    Zhang, Yanwen; Elfman, Mikael; Milbrath, Brian D.; Weber, William J.

    2008-06-26

    A recently developed fast analysis technique utilizing a time of flight (TOF) telescope is demonstrated to obtain relevant quantitative data on material scintillation response to energetic He particles. With superior energy resolution and fast response of the TOF telescope, energy of individual particle before impinging on a scintillating crystal can be determined with a high counting rate, which allows quantitative study of material performance over a continuous energy range in a relatively short time. Scintillation performances in terms of light output, nonlinearity and energy resolution in bismuth germinate (BGO) and europium-doped calcium fluoride (CaF2:Eu) Crystals are demonstrated, and the corresponding energy resolution is compared with gamma-ray tests on the same crystals.

  6. Scintillator plate calorimetry

    SciTech Connect

    Price, L.E.

    1990-01-01

    Calorimetry using scintillator plates or tiles alternated with sheets of (usually heavy) passive absorber has been proven over multiple generations of collider detectors. Recent detectors including UA1, CDF, and ZEUS have shown good results from such calorimeters. The advantages offered by scintillator calorimetry for the SSC environment, in particular, are speed (<10 nsec), excellent energy resolution, low noise, and ease of achieving compensation and hence linearity. On the negative side of the ledger can be placed the historical sensitivity of plastic scintillators to radiation damage, the possibility of nonuniform response because of light attenuation, and the presence of cracks for light collection via wavelength shifting plastic (traditionally in sheet form). This approach to calorimetry is being investigated for SSC use by a collaboration of Ames Laboratory/Iowa State University, Argonne National Laboratory, Bicron Corporation, Florida State University, Louisiana State University, University of Mississippi, Oak Ridge National Laboratory, Virginia Polytechnic Institute and State University, Westinghouse Electric Corporation, and University of Wisconsin.

  7. Scintillation spectrometry with HgI/sub 2/ as the photodetector

    SciTech Connect

    Iwanczyk, J.S.; Barton, J.B.; Dabrowski, A.J.; Kusmiss, J.H.; Szymczyk, W.M.; Huth, G.C.; Markakis, J.; Schnepple, W.F.; Lynn, R.

    1982-01-01

    A mercuric iodide (HgI/sub 2/) photodetector has been used to detect light pulses from gamma-ray and alpha-particle interactions in scintillators. The photocurrent response of an HgI/sub 2/ photodetector to light has been measured and found to be favorable for detecting light from most scintillators, which have their maximum emission between 300 and 500 nm. Energy spectra for alpha particles or gamma-rays from combinations of an HgI/sub 2/ photodetector with various scintillators are presented. The energy resolution of the photopeak from annihilation gamma-rays is 19% with a CsI(Tl) crystal and 24% with a BGO crystal. Fabrication of HgI/sub 2/ photodetectors and their optical coupling to a scintillator crystal are described. The advantages of this new solid-state radiation detector compared to the combination of scintillator and PMT, and some proposed applications, are discussed.

  8. Chloride, bromide and iodide scintillators with europium

    DOEpatents

    Zhuravleva, Mariya; Yang, Kan

    2016-09-27

    A halide scintillator material is disclosed where the halide may comprise chloride, bromide or iodide. The material is single-crystalline and has a composition of the general formula ABX.sub.3 where A is an alkali, B is an alkali earth and X is a halide which general composition was investigated. In particular, crystals of the formula ACa.sub.1-yEu.sub.yI.sub.3 where A=K, Rb and Cs were formed as well as crystals of the formula CsA.sub.1-yEu.sub.yX.sub.3 (where A=Ca, Sr, Ba, or a combination thereof and X=Cl, Br or I or a combination thereof) with divalent Europium doping where 0.ltoreq.y.ltoreq.1, and more particularly Eu doping has been studied at one to ten mol %. The disclosed scintillator materials are suitable for making scintillation detectors used in applications such as medical imaging and homeland security.

  9. Scintillator Waveguide For Sensing Radiation

    DOEpatents

    Bliss, Mary; Craig, Richard A.; Reeder; Paul L.

    2003-04-22

    The present invention is an apparatus for detecting ionizing radiation, having: a waveguide having a first end and a second end, the waveguide formed of a scintillator material wherein the therapeutic ionizing radiation isotropically generates scintillation light signals within the waveguide. This apparatus provides a measure of radiation dose. The apparatus may be modified to permit making a measure of location of radiation dose. Specifically, the scintillation material is segmented into a plurality of segments; and a connecting cable for each of the plurality of segments is used for conducting scintillation signals to a scintillation detector.

  10. Scintillator requirements for medical imaging

    SciTech Connect

    Moses, William W.

    1999-09-01

    Scintillating materials are used in a variety of medical imaging devices. This paper presents a description of four medical imaging modalities that make extensive use of scintillators: planar x-ray imaging, x-ray computed tomography (x-ray CT), SPECT (single photon emission computed tomography) and PET (positron emission tomography). The discussion concentrates on a description of the underlying physical principles by which the four modalities operate. The scintillator requirements for these systems are enumerated and the compromises that are made in order to maximize imaging performance utilizing existing scintillating materials are discussed, as is the potential for improving imaging performance by improving scintillator properties.

  11. Boron loaded scintillator

    SciTech Connect

    Bell, Zane William; Brown, Gilbert Morris; Maya, Leon; Sloop, Jr., Frederick Victor; Sloop, Jr., Frederick Victor

    2009-10-20

    A scintillating composition for detecting neutrons and other radiation comprises a phenyl containing silicone rubber with carborane units and at least one phosphor molecule. The carbonate units can either be a carborane molecule dispersed in the rubber with the aid of a compatibilization agent or can be covalently bound to the silicone.

  12. Polysiloxane scintillator composition

    DOEpatents

    Walker, J.K.

    1992-05-05

    A plastic scintillator useful for detecting ionizing radiation comprising a matrix which comprises an optically transparent polysiloxane having incorporated therein at least one ionizing radiation-hard fluor capable of converting electromagnetic energy produced in the polysiloxane upon absorption of ionizing radiation to detectable light.

  13. Polysiloxane scintillator composition

    DOEpatents

    Walker, James K.

    1992-01-01

    A plastic scintillator useful for detecting ionizing radiation comprising a matrix which comprises an optically transparent polysiloxane having incorporated therein at least one ionizing radiation-hard fluor capable of converting electromagnetic energy produced in the polysiloxane upon absorption of ionizing radiation to detectable light.

  14. Quenching equation for scintillation

    NASA Astrophysics Data System (ADS)

    Kato, Takahisa

    1980-06-01

    A mathematical expression is postulated showing the relationship between counting rate and quenching agent concentration in a liquid scintillation solution. The expression is more suited to a wider range of quenching agent concentrations than the Stern-Volmer equation. An estimation of the quenched correction is demonstrated using the expression.

  15. Transparent Ceramic Scintillator Fabrication, Properties and Applications

    SciTech Connect

    Cherepy, N J; Kuntz, J D; Roberts, J J; Hurst, T A; Drury, O B; Sanner, R D; Tillotson, T M; Payne, S A

    2008-08-24

    Transparent ceramics offer an alternative to single crystals for scintillator applications such as gamma ray spectroscopy and radiography. We have developed a versatile, scaleable fabrication method, using Flame Spray Pyrolysis (FSP) to produce feedstock which is readily converted into phase-pure transparent ceramics. We measure integral light yields in excess of 80,000 Ph/MeV with Cerium-doped Garnets, and excellent optical quality. Avalanche photodiode readout of Garnets provides resolution near 6%. For radiography applications, Lutetium Oxide offers a high performance metric and is formable by ceramics processing. Scatter in transparent ceramics due to secondary phases is the principal limitation to optical quality, and afterglow issues that affect the scintillation performance are presently being addressed.

  16. Development of High-Resolution Scintillator Systems

    SciTech Connect

    Larry A. Franks; Warnick J. Kernan

    2007-09-01

    Mercuric iodide (HgI2) is a well known material for the direct detection of gamma-rays; however, the largest volume achievable is limited by the thickness of the detector which needs to be a small fraction of the average trapping length for electrons. We report results of using HgI2 crystals to fabricate photocells used in the readout of scintillators. The optical spectral response and efficiency of these photocells were measured and will be reported. Nuclear response from an HgI2 photocell that was optically matched to a cerium-activated scintillator is presented and discussed. Further improvements can be expected by optimizing the transparent contact technology.

  17. Scintillation Properties of Eu2+-Activated Barium Fluoroiodide

    SciTech Connect

    Gundiah, Gautam; Bourret-Courchesne, Edith; Bizarri, Gregory; Hanrahan, Stephen M.; Chaudhry, Anurag; Canning, Andrew; Moses, William W.; Derenzo, Stephen E.

    2009-11-18

    The scintillation properties of powders and single-crystals of BaFI doped with Eu2+ are presented. Single crystals were grown by the vertical Bridgman technique. Under optical and X-ray excitation, the samples exhibit a narrow E2+ 5d-4f transition emission centered at 405 nm. The scintillation light output is estimated to be 55,000+-5,000 photons/MeV at 662 keV with 85percent of the light decaying within 600 ns. An energyresolution of 8.5percent full width at half maximum (FWHM) has been achieved using this scintillator for 662 keV excitation (137Cs source) at room temperature.

  18. Proton-induced radioactivity in NaI (Tl) scintillation detectors

    NASA Technical Reports Server (NTRS)

    Fishman, G. J.

    1977-01-01

    Radioactivity induced by protons in sodium iodide scintillation crystals were calculated and directly measured. These data are useful in determining trapped radiation and cosmic-ray induced, background-counting rates in spaceborne detectors.

  19. Composite scintillator screen

    DOEpatents

    Zeman, Herbert D.

    1994-01-01

    A scintillator screen for an X-ray system includes a substrate of low-Z material and bodies of a high-Z material embedded within the substrate. By preselecting the size of the bodies embedded within the substrate, the spacial separation of the bodies and the thickness of the screen, the sensitivity of the screen to X-rays within a predetermined energy range can be predicted.

  20. Ca2+-Doped CeBr3 Scintillating Materials

    SciTech Connect

    Guss, Paul; Foster, Michael E.; Wong, Bryan M.; Doty, F. Patrick; Shah, Kanai; Squillante, Michael R.; Shirwadkar, Urmila; Hawrami, Rastgo; Tower, Josh; Yuan, Ding

    2014-01-01

    Despite the outstanding scintillation performance characteristics of cerium tribromide (CeBr3) and cerium-activated lanthanum tribromide, their commercial availability and application are limited due to the difficulties of growing large, crack-free single crystals from these fragile materials. This investigation employed aliovalent doping to increase crystal strength while maintaining the optical properties of the crystal. One divalent dopant (Ca2+) was used as a dopant to strengthen CeBr3 without negatively impacting scintillation performance. Ingots containing nominal concentrations of 1.9% of the Ca2+ dopant were grown. Preliminary scintillation measurements are presented for this aliovalently doped scintillator. Ca2+-doped CeBr3 exhibited little or no change in the peak fluorescence emission for 371 nm optical excitation for CeBr3. The structural, electronic, and optical properties of CeBr3 crystals were studied using the density functional theory within the generalized gradient approximation. The calculated lattice parameters are in good agreement with the experimental data. The energy band structures and density of states were obtained. The optical properties of CeBr3, including the dielectric function, were calculated.

  1. Counterintuitive MCNPX Results for Scintillator Surface Roughness Effect

    SciTech Connect

    Yuan, Ding; Guss, Paul

    2012-10-01

    We performed a number of comparative MCNPX simulations of gamma energy depositions of scintillation crystals with smooth and rough surfaces. In the study, nine surface patterns (8 micro-roughness + 1 smooth) were coupled with eight common scintillation crystals for a total of 72 possible combinations. Although this was a preliminary study, the outcome was counterintuitive; results generally favored surfaces with micro-roughness over a conventional smooth surface as measured in terms of average energy depositions. The advantage gained through surface roughness is less significant for CdSe and LaCl3, but is most significant for the common NaI and the glass-like SiO2 scintillators. Based on the results of the 64 rough-surface coupled MCNPX simulations, 57 of the 64 (~89%) simulations showed some improvement in energy deposition. The mean improvement in energy deposition was 2.52%. The maximum improvement was about 8.75%, which was achieved when roughening the surface of a SiO2 scintillator using a micro cutting pattern. Further, for a conventional NaI scintillator, MCNPX results suggest that any roughness pattern would improve the energy deposition, with an average improvement of 3.83%. Although the likely causes remain unclear, we intend to focus on presenting simulation results instead of offering a sound explanation of the underlying physics.

  2. Cerium fluoride, a new fast, heavy scintillator

    SciTech Connect

    Moses, W.W.; Derenzo, S.E.

    1988-11-01

    We describe the scintillation properties of Cerium Fluoride (CeF/sub 3/), a newly discovered, heavy (6.16 g/cm/sup 3/), inorganic scintillator. Its fluorescence decay lifetime, measured with the delayed coincidence method, is described by a single exponential with a 27 /+-/ ns time constant. The emission spectrum peaks at a wavelength of 340 nm, and drops to less than 10% of its peak value at 315 nm and 460 nm. When a 1 cm optical quality cube of CeF/sub 3/ is excited with 511 keV photons, a photopeak with a 20% full width at half maximum is observed at approximately half the light output of a Bismuth Germanate (BGO) crystal with similar geometry. We also present measurements of the decay time and light output of CeF/sub 3/ doped with three rare-earth elements (Dy, Er, and Pr). The short fluorescence lifetime, high density, and reasonable light output of this new scintillator suggest that it would be useful for applications where high counting rates, good stopping power, and nanosecond timing are important, such as medical imaging and nuclear science. 5 refs., 6 figs., 1 tab.

  3. Neutron crosstalk between liquid scintillators

    SciTech Connect

    Verbeke, J. M.; Prasad, M. K.; Snyderman, N. J.

    2015-05-01

    We propose a method to quantify the fractions of neutrons scattering between liquid scintillators. Using a spontaneous fission source, this method can be utilized to quickly characterize an array of liquid scintillators in terms of crosstalk. The point model theory due to Feynman is corrected to account for these multiple scatterings. Using spectral information measured by the liquid scintillators, fractions of multiple scattering can be estimated, and mass reconstruction of fissile materials under investigation can be improved. Monte Carlo simulations of mono-energetic neutron sources were performed to estimate neutron crosstalk. A californium source in an array of liquid scintillators was modeled to illustrate the improvement of the mass reconstruction.

  4. Neutron crosstalk between liquid scintillators

    NASA Astrophysics Data System (ADS)

    Verbeke, J. M.; Prasad, M. K.; Snyderman, N. J.

    2015-09-01

    A method is proposed to quantify the fractions of neutrons scattering between liquid scintillators. Using a spontaneous fission source, this method can be utilized to quickly characterize an array of liquid scintillators in terms of crosstalk. The point model theory due to Feynman is corrected to account for these multiple scatterings. Using spectral information measured by the liquid scintillators, fractions of multiple scattering can be estimated, and mass reconstruction of fissile materials under investigation can be improved. Monte Carlo simulations of mono-energetic neutron sources were performed to estimate neutron crosstalk. A californium source in an array of liquid scintillators was modeled to illustrate the improvement of the mass reconstruction.

  5. New Cerium-Based Metal-Organic Scintillators for Radiation Detection

    SciTech Connect

    Boatner, Lynn A; Neal, John S; Ramey, Joanne Oxendine; Chakoumakos, Bryan C; Custelcean, Radu; Van Loef, Edgar; Markosyan, G

    2013-01-01

    We have previously shown that a new class of scintillating materials can be developed based on the synthesis and crystal growth of rare-earth metal-organic compounds. The first scintillator of this type consisted of single crystals of CeCl3(CH3OH)4 that were grown from a methanol solution. These crystals were shown to be applicable to both gamma-ray and fast neutron detection. Subsequently, metal-organic scintillators consisting of the compound LaBr3(CH3OH)4 activated with varying levels of Ce3+ and of CeBr3(CH3OH)4 were grown in single crystal form. We have now extended the development of this new class of scintillators to more complex organic components by reacting rare-earth halides such as CeCl3 or CeBr3 with different isomers of propanol and butanol including 1-propanol, isobutanol, n-butanol, and tert-butanol. The reaction of CeCl3 or CeBr3 with these organics results in the formation of new and relatively complex molecular crystals whose structures were determined using single-crystal X-ray diffraction. These new metal-organic scintillating materials were grown in single crystal form from solution, and their scintillation characteristics have been investigated using X-ray-excited luminescence plus energy spectra obtained with gamma-ray and alpha-particle sources. If the reactions between the inorganic and organic components are not carried out under very dry and highly controlled conditions, molecular structures can be formed that incorporate waters of hydration. The present observation of scintillation in these hydrated rare-earth metal-organic compounds is apparently an original finding, since we are not aware of any previous reports of scintillation being observed in a material that incorporates waters of hydration

  6. The First Tests of a Large-Area Light Detector Equipped with Metallic Magnetic Calorimeters for Scintillating Bolometers for the LUMINEU Neutrinoless Double Beta Decay Search

    NASA Astrophysics Data System (ADS)

    Gray, D.; Enss, C.; Fleischmann, A.; Gastaldo, L.; Hassel, C.; Hengstler, D.; Kempf, S.; Loidl, M.; Navick, X. F.; Rodrigues, M.

    2016-08-01

    Future rare-event searches using scintillating crystals need very low background levels for high sensitivity; however, unresolved pile-up can limit this. We present the design and fabrication of large-area photon detectors based on metallic magnetic calorimeters (MMCs), optimized for fast rise times to resolve close pile-up. The first prototypes have been characterized using Fe-55 X-rays and ZnMoO4 crystal scintillation light. A fast intrinsic rise time of 25-30 \\upmu s has been measured and has been compared to the 250 \\upmu s scintillation light pulse rise time constant. The difference indicates that the scintillation process limits the light pulse rise time. The fast rise time allows for a reduction of background due to close pile-up events as well as the study of the inherent crystal scintillation process. MMC-based photon detectors are shown to be a promising tool for scintillating crystal based rare event searches.

  7. Bismuth germanate as a potential scintillation detector in positron cameras.

    PubMed

    Cho, Z H; Farukhi, M R

    1977-08-01

    Timing and energy resolutions of the bismuth germanate (Bi4Ge3O12) scintillation crystals were studied, with particular respect to a positron-camera application. In comparison with the NaI(Tl) system, the detection efficiency for annihilation radiation is more than triple, and coincidence detection efficiency is more than ten times as good. This paper explores the properties of the new scintillator material and their bearing on the spatial resolution and the efficiency of coincidence detection in positron cameras with stationary ring detectors.

  8. Characterization of a SrF2 Scintillating Bolometer

    NASA Astrophysics Data System (ADS)

    Ginestra, C.; Coron, N.; García, E.; de Marcillac, P.; Martínez, M.; Ortigoza, Y.; Redon, T.; Torres, L.

    2012-06-01

    We present the analysis of the data obtained with a 53 g SrF2 scintillating bolometer operated at 20 mK. We have analyzed its heat and light response (time constants, linearity and energy resolution) and measured its scintillation relative efficiency factor for different particles (alpha, beta/gamma and neutrons). We have studied the spatial uniformity of the light output profiting from its internal contamination. The light amplitude of alphas from the delayed coincidence 224Ra→220Rn→216Po (emitted from the same crystal position) shows a positive correlation, evidence of a non-uniformity that worsens the light signal energy resolution by more than 50%.

  9. SU-C-201-01: Investigation of the Effects of Scintillator Surface Treatment On Light Output Measurements with SiPM Detectors

    SciTech Connect

    Valenciaga, Y; Prout, D; Chatziioannou, A

    2015-06-15

    Purpose: To examine the effect of different scintillator surface treatments (BGO crystals) on the fraction of scintillation photons that exit the crystal and reach the photodetector (SiPM). Methods: Positron Emission Tomography is based on the detection of light that exits scintillator crystals, after annihilation photons deposit energy inside these crystals. A considerable fraction of the scintillation light gets trapped or absorbed after going through multiple internal reflections on the interfaces surrounding the crystals. BGO scintillator crystals generate considerably less scintillation light than crystals made of LSO and its variants. Therefore, it is crucial that the small amount of light produced by BGO exits towards the light detector. The surface treatment of scintillator crystals is among the factors affecting the ability of scintillation light to reach the detectors. In this study, we analyze the effect of different crystal surface treatments on the fraction of scintillation light that is detected by the solid state photodetector (SiPM), once energy is deposited inside a BGO crystal. Simulations were performed by a Monte Carlo based software named GATE, and validated by measurements from individual BGO crystals coupled to Philips digital-SiPM sensor (DPC-3200). Results: The results showed an increment in light collection of about 4 percent when only the exit face of the BGO crystal, is unpolished; compared to when all the faces are polished. However, leaving several faces unpolished caused a reduction of at least 10 percent of light output when the interaction occurs as far from the exit face of the crystal as possible compared to when it occurs very close to the exit face. Conclusion: This work demonstrates the advantages on light collection from leaving unpolished the exit face of BGO crystals. The configuration with best light output will be used to obtain flood images from BGO crystal arrays coupled to SiPM sensors.

  10. GPS Scintillation Analysis.

    DTIC Science & Technology

    2007-11-02

    Rev. 2-89) Prescribed by ANSI Std. Z39-1 298-102 TABLE OF CONTENTS 1. INTRODUCTION 1 2. GPS COMPARISON WITH ALL-SKY IMAGES OVER AGUA VERDE...Depletions from 1 October 1994 2 3. GPS data from Agua Verde, Chile on the night of 1 October 1994 3 4. PL-SCINDA display of GPS ionospheric...comparison of GPS measurements with GOES8 L-band scintillation data, are discussed. 2. GPS COMPARISON WITH ALL-SKY IMAGES OVER AGUA VERDE, CHILE As

  11. Using Thin Films to Screen Possible Scintillator Materials

    SciTech Connect

    Milbrath, Brian D.; Caggiano, Joseph A.; Engelhard, Mark H.; Joly, Alan G.; Matson, Dean W.; Nachimuthu, Ponnusamy; Olsen, Larry C.

    2009-06-30

    The discovery and optimization of new scintillators has traditionally been a rather slow process due to the difficulties of single crystal growth. This paper discusses the production of polycrystalline scintillator thin films (a few microns thick) which were tested in order to determine what characterizations could be made concerning a material’s ultimate potential as a scintillator prior to pursuing crystal growth. Thin films of CaF2(Eu), CeF3, and CeCl3, all known scintillators, were produced by vapor deposition. The hygroscopic CeCl3 was coated with multiple polymer-aluminum oxide bi-layers. Emission spectra peak wavelengths and decay times agreed with single crystal values. The films were too thin to measure gamma photopeaks, but using alpha energy deposition peaks, one could compare the relative photon yield/MeV between materials. The values obtained appear to give a relevant indication of a material’s light yield potential. The technique also appears useful for quickly determining the proper dopant amount for a given material.

  12. New Scintillator Materials (K2CeBr5) and (Cs2CeBr5)

    NASA Technical Reports Server (NTRS)

    Hawrami, R.; Volz, M. P.; Batra, A. K.; Aggarwal, M. D.; Roy, U. N.; Groza, M.; Burger, A.; Cherepy, Nerine; Niedermayr, Thomas; Payne, Stephen A.

    2008-01-01

    Cesium cerium bromide (Cs2CeBr5) and potassium cerium bromide (K2CeBr5) are new scintillator materials for X-ray and gamma ray detector applications. Recently halide scintillator materials, such as Ce doped lanthanum bromide has been proved to be very important material for the same purpose. These materials are highly hygroscopic; a search for high light yield non-hygroscopic materials was highly desirable to advance the scintillator technology. In this paper, we are reporting the crystal growth of novel scintillator materials, cesium cerium bromide (Cs2CeBr5) and potassium cerium bromide (K2CeBr5). Crystals were successfully grown from the melt using the vertical Bridgman-Stockbarger technique, in a comparison with the high performance LaBr3 or LaCl3 crystals, cerium based alkali halides crystals, (Cs2CeBr5) and (K2CeBr5) have similar scintillation properties, while being much less hygroscopic. Furthermore, cesium based compounds will not suffer from the self-activity present in potassium and lanthanum compounds. However the Cs2CeBr5 crystals did not grow properly probably due to non-congruent melting or to some phase transition during cooling. Keywords." Scintillator materials; Ce3+; Energy resolution; Light yield; K2CeBr5

  13. Scintillation detector for carbon-14

    NASA Technical Reports Server (NTRS)

    Knoll, G. F.; Rogers, W. L.

    1971-01-01

    Detector consists of plastic, cylindrical double-wall scintillation cell, which is filled with gas to be analyzed. Thin, inner cell wall is isolated optically from outer (guard) scintillator wall by evaporated-aluminum coating. Bonding technique provides mechanical support to cell wall when device is exposed to high temperatures.

  14. Development of radiation hard scintillators

    SciTech Connect

    Markley, F.; Davidson, M.; Keller, J.; Foster, G.; Pla-Dalmau, A.; Harmon, J.; Biagtan, E.; Schueneman, G.; Senchishin, V.; Gustfason, H.; Rivard, M.

    1993-11-01

    The authors have demonstrated that the radiation stability of scintillators made from styrene polymer is very much improved by compounding with pentaphenyltrimethyltrisiloxane (DC 705 vacuum pump oil). The resulting scintillators are softer than desired, so they decided to make the scintillators directly from monomer where the base resin could be easily crosslinked to improve the mechanical properties. They can now demonstrate that scintillators made directly from the monomer, using both styrene and 4-methyl styrene, are also much more radiation resistant when modified with DC705 oil. In fact, they retain from 92% to 95% of their original light output after gamma irradiation to 10 Mrads in nitrogen with air annealing. When these scintillators made directly from monomer are compared with scintillators of the same composition made from polymer the latter have much higher light outputs. They commonly reach 83% while those made form monomer give only 50% to 60% relative to the reference, BC408. When oil modified scintillators using both p-terphenyl and tetraphenylbutadiene are compared with identical scintillators except that they use 3 hydroxy-flavone as the only luminophore the radiation stability is the same. However the 3HF system gives only 30% as much light as BC408 instead of 83% when both are measured with a green extended Phillips XP2081B phototube.

  15. Hybrid scintillators for neutron discrimination

    DOEpatents

    Feng, Patrick L; Cordaro, Joseph G; Anstey, Mitchell R; Morales, Alfredo M

    2015-05-12

    A composition capable of producing a unique scintillation response to neutrons and gamma rays, comprising (i) at least one surfactant; (ii) a polar hydrogen-bonding solvent; and (iii) at least one luminophore. A method including combining at least one surfactant, a polar hydrogen-bonding solvent and at least one luminophore in a scintillation cell under vacuum or an inert atmosphere.

  16. Extruding plastic scintillator at Fermilab

    SciTech Connect

    Anna Pla-Dalmau; Alan D. Bross; Victor V. Rykalin

    2003-10-31

    An understanding of the costs involved in the production of plastic scintillators and the development of a less expensive material have become necessary with the prospects of building very large plastic scintillation detectors. Several factors contribute to the high cost of plastic scintillating sheets, but the principal reason is the labor-intensive nature of the manufacturing process. In order to significantly lower the costs, the current casting procedures had to be abandoned. Since polystyrene is widely used in the consumer industry, the logical path was to investigate the extrusion of commercial-grade polystyrene pellets with dopants to yield high quality plastic scintillator. This concept was tested and high quality extruded plastic scintillator was produced. The D0 and MINOS experiments are already using extruded scintillator strips in their detectors. An extrusion line has recently been installed at Fermilab in collaboration with NICADD (Northern Illinois Center for Accelerator and Detector Development). This new facility will serve to further develop and improve extruded plastic scintillator. This paper will discuss the characteristics of extruded plastic scintillator and its raw materials, the different manufacturing techniques and the current R&D program at Fermilab.

  17. Development of intrinsic IPT scintillator

    SciTech Connect

    Bross, A.D.

    1989-07-31

    We report on the development of a new polystyrene based plastic scintillator. Optical absorption, fluorescence and light output measurements are presented. Preliminary results of radiation damage effects are also given and compared to the effects on a commercial plastic scintillator, NE 110. 6 refs., 12 figs.

  18. Efficiency of Scintillator Materials in the Energy Range 8.0-32.0 keV

    SciTech Connect

    Kinney, J H; Haupt, D L

    2002-07-01

    X-ray microtomography requires the measurement of x-ray attenuation along ray paths through a specimen, and on the inversion of these data to obtain a spatially resolved mapping of the microstructure of the specimen. To do this efficiently, two-dimensional array detectors are often used to measure the transmitted x-rays by capturing and recording each x-ray incident on the detector. The highest resolution CT instruments perform this by converting the incident x-rays to visible light, and then focusing this light onto a charge-coupled-device (CCD) detector. The light output of the scintillator (photons per incident x-ray), the numerical aperture of the optical lens system, and the quantum efficiency of the CCD govern the efficiency of the detection process. Several years earlier, our group performed an investigation aimed at determining the best scintillator material for high-resolution synchrotron CT. The selection criteria included light output in the 8-32 keV energy range, the spatial resolution of the scintillator, the wavelength of the scintillation radiation, and the stability and ease of polishing of the scintillator. A list of the scintillators that we considered, with the exceptions of the more recently developed glass scintillators, is provided in Table 1. Among these scintillators, we concluded that single crystal cadmium tungstate was optimum; we have used this material in all subsequent synchrotron CT systems. Since this original study, several doped-glass scintillators have become available. The LSO (Lu orthosilicates) scintillators, developed for PET scanning, show considerable light output at high energy (energies above 500 keV). Theoretically, the light output of these scintillators should be twice that of the cadmium tungstate. The purpose of this study was to determine the efficiency of two such scintillators (LSO:Yt and IQI-401 high density terbium activated glass) in the energy range from 8-32 keV.

  19. Transparent BaCl II:Eu 2+ glass-ceramic scintillator

    NASA Astrophysics Data System (ADS)

    Chen, Gang; Johnson, Jacqueline; Schweizer, Stefan; Woodford, John; Newman, Peter; MacFarlane, Douglas

    2006-03-01

    Scintillators are the backbone of high-energy radiation detection devices. Most scintillators are based on inorganic crystals that have applications in medical radiography, nuclear medicine, security inspection, dosimetry, and high-energy physics. In this paper, we present a new type of scintillator that is based on glass ceramics (composites of glasses and crystals). These scintillators are made from Eu 2+-activated fluorozirconate glasses that are co-doped with Ba 2+, La 3+, Al 3+, Na +, and Cl -. Subsequent heat treatment of the glasses forms BaCl II nano-crystals (10-20 nm in size) that are embedded in the glass matrix. The resulting scintillators are transparent, efficient, inexpensive to fabricate, and easy to scale up. The physical structure and x-ray imaging performance of these glass-ceramic scintillators are presented, and an application of these materials to micro-computed tomography is demonstrated. Our study suggests that these glass-ceramic scintillators have high potential for medical x-ray imaging.

  20. DSB:Ce3+ scintillation glass for future

    NASA Astrophysics Data System (ADS)

    Auffray, E.; Akchurin, N.; Benaglia, A.; Borisevich, A.; Cowden, C.; Damgov, J.; Dormenev, V.; Dragoiu, C.; Dudero, P.; Korjik, M.; Kozlov, D.; Kunori, S.; Lecoq, P.; Lee, S. W.; Lucchini, M.; Mechinsky, V.; Pauwels, K.

    2015-02-01

    One of the main challenges for detectors at future high-energy collider experiments is the high precision measurement of hadron and jet energy and momentum. One possibility to achieve this is the dual-readout technique, which allows recording simultaneously scintillation and Cherenkov light in an active medium in order to extract the electromagnetic fraction of the total shower energy on an event- by-event basis. Making use of this approach in the high luminosity LHC, however, puts stringent requirements on the active materials in terms of radiation hardness. Consequently, the R&D carried out on suitable scintillating materials focuses on the detector performance as well as on radiation tolerance. Among the different scintillating materials under study, scintillating glasses can be a suitable solution due to their relatively simple and cost effective production. Recently a new type of inorganic scintillating glass: Cerium doped DSB has been developed by Radiation Instruments and New Components LLC in Minsk for oil logging industry. This material can be produced either in form of bulk or fiber shape with diameter 0.3-2mm and length up to 2000 mm. It is obtained by standard glass production technology at temperature 1400°C with successive thermal annealing treatment at relatively low temperature. The production of large quantities is relatively easy and the production costs are significantly lower compared to crystal fibers. Therefore, this material is considered as an alternative and complementary solution to crystal fibers in view of a production at industrial scale, as required for a large dual readout calorimeter. In this paper, the first results on optical, scintillation properties as well as the radiation damage behaviour obtained on different samples made with different raw materials and various cerium concentrations will be presented.

  1. Maximum likelihood positioning and energy correction for scintillation detectors.

    PubMed

    Lerche, Christoph W; Salomon, André; Goldschmidt, Benjamin; Lodomez, Sarah; Weissler, Björn; Solf, Torsten

    2016-02-21

    An algorithm for determining the crystal pixel and the gamma ray energy with scintillation detectors for PET is presented. The algorithm uses Likelihood Maximisation (ML) and therefore is inherently robust to missing data caused by defect or paralysed photo detector pixels. We tested the algorithm on a highly integrated MRI compatible small animal PET insert. The scintillation detector blocks of the PET gantry were built with the newly developed digital Silicon Photomultiplier (SiPM) technology from Philips Digital Photon Counting and LYSO pixel arrays with a pitch of 1 mm and length of 12 mm. Light sharing was used to readout the scintillation light from the 30 × 30 scintillator pixel array with an 8 × 8 SiPM array. For the performance evaluation of the proposed algorithm, we measured the scanner's spatial resolution, energy resolution, singles and prompt count rate performance, and image noise. These values were compared to corresponding values obtained with Center of Gravity (CoG) based positioning methods for different scintillation light trigger thresholds and also for different energy windows. While all positioning algorithms showed similar spatial resolution, a clear advantage for the ML method was observed when comparing the PET scanner's overall single and prompt detection efficiency, image noise, and energy resolution to the CoG based methods. Further, ML positioning reduces the dependence of image quality on scanner configuration parameters and was the only method that allowed achieving highest energy resolution, count rate performance and spatial resolution at the same time.

  2. Radiation-resistant composite scintillators based on GSO and GPS grains

    NASA Astrophysics Data System (ADS)

    Boyarintsev, A. Yu.; Galunov, N. Z.; Gerasymov, Ia. V.; Karavaeva, N. L.; Krech, A. V.; Levchuk, L. G.; Popov, V. F.; Sidletskiy, O. Ts.; Sorokin, P. V.; Tarasenko, O. A.

    2017-01-01

    The effect of irradiation on the scintillation light output, optical transmittance, and luminescent spectra of composite scintillators based on grains of single crystals Gd2SiO5:Ce (GSO) and Gd2Si2O7:Ce (GPS) is studied. The dielectric gel Sylgard-184 is the base and the binder for the grains inside the composite scintillator. The paper presents and analyzes the results obtained for the scintillators exposed by 10 MeV electrons from the linear electron accelerator at room temperature. The exposure doses D≤250 Mrad. The dose rate is 0.2 or 1500 Mrad/h. The study has shown that the composite scintillators based on the grains of GSO and GPS are radiation-resistant over the range of the irradiation.

  3. High resolution scintillation spectroscopy with HgI/sub 2/ as the photodetector

    SciTech Connect

    Markakis, J.M.

    1987-01-01

    This report details the progress made in developing mercuric iodide photocells - in particular as the photodetector in scintillation spectrometers where photomultipliers are conventionally used. A spectrometer consisting of an HgI/sub 2/ photocell optically coupled with a CsI(Tl) scintillator gave a /sup 137/Cs (662 keV) resolution of 5.33% FWHM, the best /sup 137/Cs resolution reported to date using a scintillation spectrometer. Relative to photomultiplier tubes, solid state photodetectors are smaller, insensitive to magnetic fields, and have higher quantum efficiencies. HgI/sub 2/ photocells offer an unprecedented energy resolution for scintillation spectrometers and push closer to the resolution of scintillation crystals themselves.

  4. Proton recoil scintillator neutron rem meter

    DOEpatents

    Olsher, Richard H.; Seagraves, David T.

    2003-01-01

    A neutron rem meter utilizing proton recoil and thermal neutron scintillators to provide neutron detection and dose measurement. In using both fast scintillators and a thermal neutron scintillator the meter provides a wide range of sensitivity, uniform directional response, and uniform dose response. The scintillators output light to a photomultiplier tube that produces an electrical signal to an external neutron counter.

  5. Effect of host glass matrix on structural and optical behavior of glass-ceramic nanocomposite scintillators

    NASA Astrophysics Data System (ADS)

    Brooke Barta, M.; Nadler, Jason H.; Kang, Zhitao; Wagner, Brent K.; Rosson, Robert; Kahn, Bernd

    2013-12-01

    Composite scintillator systems have received increased attention in recent years due to their promise for merging the radioisotope discrimination capabilities of single crystal scintillators with the high throughput scanning capabilities of portal monitors. However, producing the high light yield required for good energy resolution has proven challenging as scintillation photons are often scattered by variations in refractive index and agglomerated scintillator crystals within the composite. This investigation sought to mitigate these common problems by using glass-ceramic nanocomposite materials systems in which nanoscale scintillating crystallites are precipitated in a controlled manner from a transparent glass matrix. Precipitating crystallites in situ precludes nanoparticle agglomeration, and limiting crystallite size to 50 nm or less mitigates the effect of refractive index mismatch between the crystals and host glass. Cerium-doped gadolinium bromide (GdBr3(Ce)) scintillating crystals were incorporated into sodium-aluminosilicate (NAS) and alumino-borosilicate (ABS) host glass matrices, and the resulting glass-ceramic structures and luminescence behavior were characterized. The as-cast glass from the ABS system displayed a highly ordered microstructure that produced the highest luminescence intensity (light yield) of the samples studied. However, heat treating to form the glass-ceramic precipitated rare-earth oxide crystallites rather than rare-earth halides. This degraded light yield relative to the unaged sample.

  6. Liquid scintillator tiles for calorimetry

    SciTech Connect

    Amouzegar, M.; Belloni, A.; Bilki, B.; Calderon, J.; Barbaro, P. De; Eno, S. C.; Hatakeyama, K.; Hirschauer, J.; Jeng, G. Y.; Pastika, N. J.; Pedro, K.; Rumerio, Paolo; Samuel, J.; Sharp, E.; Shin, Y. H.; Tiras, E.; Vishnevskiy, D.; Wetzel, J.; Yang, Z.; Yao, Y.; Youn, S. W.

    2016-11-28

    Future experiments in high energy and nuclear physics may require large, inexpensive calorimeters that can continue to operate after receiving doses of 50 Mrad or more. Also, the light output of liquid scintillators suffers little degradation under irradiation. However, many challenges exist before liquids can be used in sampling calorimetry, especially regarding developing a packaging that has sufficient efficiency and uniformity of light collection, as well as suitable mechanical properties. We present the results of a study of a scintillator tile based on the EJ-309 liquid scintillator using cosmic rays and test beam on the light collection efficiency and uniformity, and some preliminary results on radiation hardness.

  7. Liquid scintillator tiles for calorimetry

    NASA Astrophysics Data System (ADS)

    Amouzegar, M.; Belloni, A.; Bilki, B.; Calderon, J.; De Barbaro, P.; Eno, S. C.; Hatakeyama, K.; Hirschauer, J.; Jeng, G. Y.; Pastika, N. J.; Pedro, K.; Rumerio, Paolo; Samuel, J.; Sharp, E.; Shin, Y. H.; Tiras, E.; Vishnevskiy, D.; Wetzel, J.; Yang, Z.; Yao, Y.; Youn, S. W.

    2016-11-01

    Future experiments in high energy and nuclear physics may require large, inexpensive calorimeters that can continue to operate after receiving doses of 50 Mrad or more. The light output of liquid scintillators suffers little degradation under irradiation. However, many challenges exist before liquids can be used in sampling calorimetry, especially regarding developing a packaging that has sufficient efficiency and uniformity of light collection, as well as suitable mechanical properties. We present the results of a study of a scintillator tile based on the EJ-309 liquid scintillator using cosmic rays and test beam on the light collection efficiency and uniformity, and some preliminary results on radiation hardness.

  8. Scintillator materials containing lanthanum fluorides

    DOEpatents

    Moses, William W.

    1991-01-01

    An improved radiation detector containing a crystalline mixture of LaF.sub.3 and CeF.sub.3 as the scintillator element is disclosed. Scintillators made with from 25% to 99.5% LaF.sub.3 and the remainder CeF.sub.3 have been found to provide a balance of good stopping power, high light yield and short decay constant that is equal to or superior to other known scintillator materials, and which may be processed from natural starting materials containing both rare earth elements. The radiation detectors disclosed are favorably suited for use in general purpose detection and in positron emission tomography.

  9. High energy resolution plastic scintillator

    NASA Astrophysics Data System (ADS)

    van Loef, Edgar V.; Feng, Patrick; Markosyan, Gary; Shirwadkar, Urmila; Doty, Patrick; Shah, Kanai S.

    2016-09-01

    In this paper we present results on a novel tin-loaded plastic scintillator. We will show that this particular plastic scintillator has a light output similar to that of BGO, a fast scintillation decay (< 10 ns), exhibits good neutron/gamma PSD with a Figure-of-Merit of 1.3 at 2.5 MeVee cut-off energy, and excellent energy resolution of about 12% (FWHM) at 662 keV. Under X-ray excitation, the radioluminescence spectrum exhibits a broad band between 350 and 500 nm peaking at 420 nm which is well-matched to bialkali photomultiplier tubes and UV-enhanced photodiodes.

  10. Ionospheric scintillation studies

    NASA Technical Reports Server (NTRS)

    Rino, C. L.; Freemouw, E. J.

    1973-01-01

    The diffracted field of a monochromatic plane wave was characterized by two complex correlation functions. For a Gaussian complex field, these quantities suffice to completely define the statistics of the field. Thus, one can in principle calculate the statistics of any measurable quantity in terms of the model parameters. The best data fits were achieved for intensity statistics derived under the Gaussian statistics hypothesis. The signal structure that achieved the best fit was nearly invariant with scintillation level and irregularity source (ionosphere or solar wind). It was characterized by the fact that more than 80% of the scattered signal power is in phase quadrature with the undeviated or coherent signal component. Thus, the Gaussian-statistics hypothesis is both convenient and accurate for channel modeling work.

  11. Properties of scintillator solutes

    SciTech Connect

    Fluornoy, J.M.

    1998-06-01

    This special report summarizes measurements of the spectroscopic and other properties of the solutes that were used in the preparation of several new liquid scintillators developed at EG and G/Energy Measurements/Santa Barbara Operations (the precursor to Bechtel Nevada/Special Technologies Laboratory) on the radiation-to-light converter program. The data on the individual compounds are presented in a form similar to that used by Prof. Isadore Berlman in his classic handbook of fluorescence spectra. The temporal properties and relative efficiencies of the new scintillators are presented in Table 1, and the efficiencies as a function of wavelength are presented graphically in Figure 1. In addition, there is a descriptive glossary of the abbreviations used herein. Figure 2 illustrates the basic structures of some of the compounds and of the four solvents reported in this summary. The emission spectra generally exhibit more structure than the absorption spectra, with the result that the peak emission wavelength for a given compound may lie several nm away from the wavelength, {lambda}{sub avg}, at the geometric center of the emission spectrum. Therefore, the author has chosen to list absorption peaks, {lambda}{sub max}, and emission {lambda}{sub avg} values in Figures 3--30, as being most illustrative of the differences between the compounds. The compounds, BHTP, BTPB, ADBT, and DPTPB were all developed on this program. P-terphenyl, PBD, and TPB are commercially available blue emitters. C-480 and the other longer-wavelength emitters are laser dyes available commercially from Exciton Corporation. 1 ref., 30 figs.

  12. Lithium indium diselenide: A new scintillator for neutron imaging

    DOE PAGES

    Lukosi, Eric; Herrera, Elan; Hamm, Daniel; ...

    2016-05-20

    Lithium indium diselenide, 6LiInSe2 or LISe, is a newly developed neutron detection material that shows both semiconducting and scintillating properties. The 24% atomic density of 6Li yields a thermal neutron mean free path of only 920 μm. This paper reports on the performance of LISe crystals in scintillation mode for its potential use as a converter screen for thermal/cold neutron imaging. The spatial resolution of LISe, determined using a 10% value of the Modulation Transfer Function (MTF), was found to not scale linearly with thickness. Crystals having a thickness of 450 μm or larger resulted in an average spatial resolutionmore » of 67 μm, and the thinner crystals exhibited an increase in spatial resolution down to the Nyquist frequency of the CCD. The highest measured spatial resolution of 198 μm thick LISe (27 μm) outperforms a commercial 50 μm thick ZnS(Cu):6LiF scintillation screen (100 μm) by more than a factor of three. For the thicknesses considered in this study, it has been found that the light yield of LISe did not scale with its thickness, suggesting the need for optimizing the synthesis to enhance the scintillation mechanism. Absorption measurements indicate that the 6Li concentration is uniform throughout the samples and its absorption efficiency as a function of thickness follows general nuclear theory, indicating that the variation in apparent brightness is likely due to a combination of particle escape, light transport, and activation of the scintillation mechanisms. As a result, the presence of 115In and its long-lived 116In activation product did not result in ghosting (memory of past neutron exposure), demonstrating potential for using LISe for imaging transient systems.« less

  13. Lithium indium diselenide: A new scintillator for neutron imaging

    SciTech Connect

    Lukosi, Eric; Herrera, Elan; Hamm, Daniel; Lee, Kyung -Min; Wiggins, Brenden; Trtik, Pavel; Penumadu, Dayakar; Young, Stephen; Santodonato, Louis; Bilheux, Hassina; Burger, Arnold; Matei, Liviu; Stowe, Ashley C.

    2016-05-20

    Lithium indium diselenide, 6LiInSe2 or LISe, is a newly developed neutron detection material that shows both semiconducting and scintillating properties. The 24% atomic density of 6Li yields a thermal neutron mean free path of only 920 μm. This paper reports on the performance of LISe crystals in scintillation mode for its potential use as a converter screen for thermal/cold neutron imaging. The spatial resolution of LISe, determined using a 10% value of the Modulation Transfer Function (MTF), was found to not scale linearly with thickness. Crystals having a thickness of 450 μm or larger resulted in an average spatial resolution of 67 μm, and the thinner crystals exhibited an increase in spatial resolution down to the Nyquist frequency of the CCD. The highest measured spatial resolution of 198 μm thick LISe (27 μm) outperforms a commercial 50 μm thick ZnS(Cu):6LiF scintillation screen (100 μm) by more than a factor of three. For the thicknesses considered in this study, it has been found that the light yield of LISe did not scale with its thickness, suggesting the need for optimizing the synthesis to enhance the scintillation mechanism. Absorption measurements indicate that the 6Li concentration is uniform throughout the samples and its absorption efficiency as a function of thickness follows general nuclear theory, indicating that the variation in apparent brightness is likely due to a combination of particle escape, light transport, and activation of the scintillation mechanisms. As a result, the presence of 115In and its long-lived 116In activation product did not result in ghosting (memory of past neutron exposure), demonstrating potential for using LISe for imaging transient systems.

  14. Lithium indium diselenide: A new scintillator for neutron imaging

    NASA Astrophysics Data System (ADS)

    Lukosi, Eric; Herrera, Elan; Hamm, Daniel; Lee, Kyung-Min; Wiggins, Brenden; Trtik, Pavel; Penumadu, Dayakar; Young, Stephen; Santodonato, Louis; Bilheux, Hassina; Burger, Arnold; Matei, Liviu; Stowe, Ashley C.

    2016-09-01

    Lithium indium diselenide, 6LiInSe2 or LISe, is a newly developed neutron detection material that shows both semiconducting and scintillating properties. This paper reports on the performance of scintillating LISe crystals for its potential use as a converter screen for cold neutron imaging. The spatial resolution of LISe, determined using a 10% threshold of the Modulation Transfer Function (MTF), was found to not scale linearly with thickness. Crystals having a thickness of 450 μm or larger resulted in an average spatial resolution of 67 μm, and the thinner crystals exhibited an increase in spatial resolution down to the Nyquist frequency of the CCD. The highest measured spatial resolution of 198 μm thick LISe (27 μm) outperforms a commercial 50 μm thick ZnS(Cu):6LiF scintillation screen by more than a factor of three. For the LISe dimensions considered in this study, it was found that the light yield of LISe did not scale with its thickness. However, absorption measurements indicate that the 6Li concentration is uniform and the neutron absorption efficiency of LISe as a function of thickness follows general nuclear theory. This suggests that the differences in apparent brightness observed for the LISe samples investigated may be due to a combination of secondary charged particle escape, scintillation light transport in the bulk and across the LISe-air interface, and variations in the activation of the scintillation mechanism. Finally, it was found that the presence of 115In and its long-lived 116In activation product did not result in ghosting (memory of past neutron exposure), demonstrating potential of LISe for imaging transient systems.

  15. Scintillation Characterization of Doped Cesium Hafnium Chloride (Conference Presentation)

    NASA Astrophysics Data System (ADS)

    Rowe, Emmanuel; Goodwin, Brandon; Bhattacharya, Pijush; Burger, Arnold; Stowe, Ashley; Cherepy, Nerine; Payne, Steve

    2016-09-01

    The scintillators currently providing the best energy resolution lower than 2.6% at 662 keV and sizes larger than 1 in. dia. 1 in. height are LaBr3(Ce) and SrI2(Eu). Despite energy resolution and decay time performance of LaBr3(Ce), the intrinsic radioactivity, due to naturally occurring 138La isotope in the matrix is a limitation for low count rate applications such as radioisotope identification of weak sources. Cesium Hafnium Chloride (CHC) is a high effective atomic number (Zeff=58) moderate density (3.86 g/cm3) scintillator for gamma spectroscopy, offering a cubic crystal structure, no intrinsic radioactivity, and highly proportional light yield, without intentional doping. CHC boasts a cubic crystal structure that is isostructural to K2HfCl6 and analogous to calcium fluoride with cesium ions in the fluorine ion position and the [HfCl6]2- octahedral replacing calcium ions. The scintillation of CHC is centered at 400 nm, with a principal decay time of 4.37 μs, a light yield of up to 54,000 photons/MeV and energy resolution of 3.3% at 662 keV and we report on the effects of doping on the scintillation properties of CHC.

  16. Performance of Europium-Doped Strontium Iodide, Transparent Ceramics and Bismuth-loaded Polymer Scintillators

    SciTech Connect

    Cherepy, Nerine; Payne, Stephen A.; Sturm, Benjamin; O’Neal, S P; Seeley, Zachary; Drury, Owen; Haselhorst, L K; Rupert, B. L.; Sanner, Robert; Thelin, P; Fisher, S E; Hawrami, Rastgo; Shah, Kanai; Burger, Arnold; Ramey, Joanne Oxendine; Boatner, Lynn A

    2011-01-01

    Recently discovered scintillators for gamma ray spectroscopy, single crystal SrI2(Eu), GYGAG(Ce) transparent ceramic and Bismuth-loaded plastics offer resolution and fabrication advantages compared to commercial scintillators, such as NaI(Tl) and standard PVT plastic. Energy resolution at 662 keV of 2.7% is obtained with SrI2(Eu), while 4.5% is obtained with GYGAG(Ce). A new transparent ceramic scintillator for radiographic imaging systems, GLO(Eu) offers high light yield of ~75,000 Ph/MeV, high stopping, and low radiation damage. Implementation of single crystal SrI2(Eu), Gd-based transparent ceramics, and Bi-loaded plastic scintillators can advance the state-of-the art in ionizing radiation detection systems.

  17. Application of scintillating properties of liquid xenon and silicon photomultiplier technology to medical imaging

    NASA Astrophysics Data System (ADS)

    Gomez-Cadenas, J. J.; Benlloch-Rodriguez, J. M.; Ferrario, Paola

    2016-04-01

    We describe a new positron emission time-of-flight apparatus using liquid xenon. The detector is based in a liquid xenon scintillating cell. The cell shape and dimensions can be optimized depending on the intended application. In its simplest form, the liquid xenon scintillating cell is a box in which two faces are covered by silicon photomultipliers and the others by a reflecting material such as Teflon. It is a compact, homogenous and highly efficient detector which shares many of the desirable properties of monolithic crystals, with the added advantage of high yield and fast scintillation offered by liquid xenon. Our initial studies suggest that good energy and spatial resolution comparable with that achieved by lutetium oxyorthosilicate crystals can be obtained with a detector based in liquid xenon scintillating cells. In addition, the system can potentially achieve an excellent coincidence resolving time of better than 100 ps.

  18. Performance of Europium-Doped Strontium Iodide, Transparent Ceramics and Bismuth-loaded Polymer Scintillators

    SciTech Connect

    Cherepy, N J; Payne, S A; Sturm, B W; O'Neal, S P; Seeley, Z M; Drury, O B; Haselhorst, L K; Rupert, B L; Sanner, R D; Thelin, P A; Fisher, S E; Hawrami, R; Shah, K S; Burger, A; Ramey, J O; Boatner, L A

    2011-08-30

    Recently discovered scintillators for gamma ray spectroscopy, single crystal SrI{sub 2}(Eu), GYGAG(Ce) transparent ceramic and Bismuth-loaded plastics, offer resolution and fabrication advantages compared to commercial scintillators, such as NaI(Tl) and standard PVT plastic. Energy resolution at 662 keV of 2.7% is obtained with SrI{sub 2}(Eu), while 4.5% is obtained with GYGAG(Ce). A new transparent ceramic scintillator for radiographic imaging systems, GLO(Eu) offers high light yield of 70,000 Photons/MeV, high stopping, and low radiation damage. Implementation of single crystal SrI{sub 2}(Eu), Gd-based transparent ceramics, and Bi-loaded plastic scintillators can advance the state-of-the art in ionizing radiation detection systems.

  19. Improved Growth Methods for LaBr3 Scintillation Radiation Detectors

    SciTech Connect

    McGregor, Douglas S

    2011-05-01

    The objective is to develop advanced materials for deployment as high-resolution gamma ray detectors. Both LaBr3 and CeBr3 are advanced scintillation materials, and will be studied in this research. Prototype devices, in collaboration Sandia National Laboratories, will be demonstrated along with recommendations for mass production and deployment. It is anticipated that improved methods of crystal growth will yield larger single crystals of LaBr3 for deployable room-temperature operated gamma radiation spectrometers. The growth methods will be characterized. The LaBr3 and CeBr3 scintillation crystals will be characterized for light yield, spectral resolution, and for hardness.

  20. Scintillator fiber optic long counter

    DOEpatents

    McCollum, T.; Spector, G.B.

    1994-03-29

    A flat response position sensitive neutron detector capable of providing neutron spectroscopic data utilizing scintillator fiber optic filaments embedded in a neutron moderating housing having an open end through which neutrons enter to be detected is described. 11 figures.

  1. Neutron crosstalk between liquid scintillators

    DOE PAGES

    Verbeke, J. M.; Prasad, M. K.; Snyderman, N. J.

    2015-05-01

    We propose a method to quantify the fractions of neutrons scattering between liquid scintillators. Using a spontaneous fission source, this method can be utilized to quickly characterize an array of liquid scintillators in terms of crosstalk. The point model theory due to Feynman is corrected to account for these multiple scatterings. Using spectral information measured by the liquid scintillators, fractions of multiple scattering can be estimated, and mass reconstruction of fissile materials under investigation can be improved. Monte Carlo simulations of mono-energetic neutron sources were performed to estimate neutron crosstalk. A californium source in an array of liquid scintillators wasmore » modeled to illustrate the improvement of the mass reconstruction.« less

  2. Scintillator fiber optic long counter

    DOEpatents

    McCollum, Tom; Spector, Garry B.

    1994-01-01

    A flat response position sensitive neutron detector capable of providing neutron spectroscopic data utilizing scintillator fiber optic filaments embedded in a neutron moderating housing having an open end through which neutrons enter to be detected.

  3. Combinatorial Screening of Advanced Scintillators for High Resolution X-ray Detectors

    SciTech Connect

    Cheng, Shifan; Tao, Dejie; Lynch, Michael; Yuan, Xianglong; Li, Yiqun

    2008-05-12

    The lack of efficient scintillators is a major problem for developing powerful x-ray detectors that are widely used in homeland security, industrial and scientific research. Intematix has developed and applied a high throughput screening process and corresponding crystal growth technology to significantly speed up the discovery process for new efficient scintillators. As a result, Intematix has invented and fabricated three new scintillators both in powder and bulk forms, which possess promising properties such as better radiation hardness and better matching for silicon diode.

  4. About NICADD extruded scintillating strips

    SciTech Connect

    Dyshkant, A.; Beznosko, D.; Blazey, G.; Chakraborty, D.; Francis, K.; Kubik, D.; Lima, J.G.; Rykalin, V.; Zutshi, v.; Baldina, E.; Bross, A.; Deering, P.; Nebel, T.; Pla-Dalmau, A.; Schellpfeffer, J.; Serritella, C.; Zimmerman, J.; /Fermilab

    2005-04-01

    The results of control measurements of extruded scintillating strip responses to a radioactive source Sr-90 are provided, and details of strip choice, preparation, and method of measurement are included. About four hundred one meter long extruded scintillating strips were measured at four different points. These results were essential for prototyping a tail catcher and muon tracker for a future international electron positron linear collider detector.

  5. Properties of Ce-activated alkali-lutetium double phosphate scintillators

    SciTech Connect

    Wiśniewski, D.; Wojtowicz, A. J.; Boatner, Lynn A

    2010-01-01

    The scintillation properties of Ce-activated alkali-lutetium double phosphate single crystals that vary with the alkali ion type and activation level are summarized and compared. The materials investigated here have been identified as fast and efficient scintillators for the detection of x-ray and radiation, and in case of Li3Lu(PO4)2:Ce, for thermal neutron detection as well.

  6. Methods of Fabricating Scintillators with Radioisotopes for Beta Battery Applications

    NASA Technical Reports Server (NTRS)

    Rensing, Noa M.; Squillante, Michael R.; Tieman, Timothy C.; Higgins, William; Shiriwadkar, Urmila

    2013-01-01

    Technology has been developed for a class of self-contained, long-duration power sources called beta batteries, which harvest the energy contained in the radioactive emissions from beta decay isotopes. The new battery is a significant improvement over the conventional phosphor/solar cell concept for converting this energy in three ways. First, the thin phosphor is replaced with a thick scintillator that is transparent to its own emissions. By using a scintillator sufficiently thick to completely stop all the beta particles, efficiency is greatly improved. Second, since the energy of the beta particles is absorbed in the scintillator, the semiconductor photodetector is shielded from radiation damage that presently limits the performance and lifetime of traditional phosphor converters. Finally, instead of a thin film of beta-emitting material, the isotopes are incorporated into the entire volume of the thick scintillator crystal allowing more activity to be included in the converter without self-absorption. There is no chemical difference between radioactive and stable strontium beta emitters such as Sr-90, so the beta emitter can be uniformly distributed throughout a strontium based scintillator crystal. When beta emitter material is applied as a foil or thin film to the surface of a solar cell or even to the surface of a scintillator, much of the radiation escapes due to the geometry, and some is absorbed within the layer itself, leading to inefficient harvesting of the energy. In contrast, if the emitting atoms are incorporated within the scintillator, the geometry allows for the capture and efficient conversion of the energy of particles emitted in any direction. Any gamma rays associated with secondary decays or Bremsstrahlung photons may also be absorbed within the scintillator, and converted to lower energy photons, which will in turn be captured by the photocell or photodiode. Some energy will be lost in this two-stage conversion process (high-energy particle

  7. Extruded plastic scintillator including inorganic powders

    DOEpatents

    Bross, Alan D.; Mellott, Kerry L.; Pla-Dalmau, Anna

    2006-06-27

    A method for producing a plastic scintillator is disclosed. A plurality of nano-sized particles and one or more dopants can be combined with a plastic material for the formation of a plastic scintillator thereof. The nano-sized particles, the dopant and the plastic material can be combined within the dry inert atmosphere of an extruder to produce a reaction that results in the formation of a plastic scintillator thereof and the deposition of energy within the plastic scintillator, such that the plastic scintillator produces light signifying the detection of a radiative element. The nano-sized particles can be treated with an inert gas prior to processing the nano-sized particles, the dopant and the plastic material utilizing the extruder. The plastic scintillator can be a neutron-sensitive scintillator, x-ray sensitive scintillator and/or a scintillator for the detection of minimum ionizing particles.

  8. Characterization of cerium fluoride nanocomposite scintillators

    SciTech Connect

    Stange, Sy; Esch, Ernst I; Brown, Leif O; Couture, Aaron J; Mckigney, Edward A; Muenchausen, Ross E; Del Sesto, Rico E; Gilbertson, Robert D; Mccleskey, T Mark; Reifarth, Rene

    2009-01-01

    Measurement of the neutron capture cross-sections of a number of short-lived isotopes would advance both pure and applied scientific research. These cross-sections are needed for calculation of criticality and waste production estimates for the Advanced Fuel Cycle Initiative, for analysis of data from nuclear weapons tests, and to improve understanding of nucleosynthesis. However, measurement of these cross-sections would require a detector with a faster signal decay time than those used in existing neutron capture experiments. Crystals of faster detector materials are not available in sufficient sizes and quantities to supply these large-scale experiments. Instead, we propose to use nanocomposite detectors, consisting of nanoscale particles of a scintillating material dispersed in a matrix material. We have successfully fabricated cerium fluoride (CeF{sub 3}) nanoparticles and dispersed them in a liquid matrix. We have characterized this scintillator and have measured its response to neutron capture. Results of the optical, structural, and radiation characterization will be presented.

  9. Performance of photomultiplier tubes and sodium iodide scintillation detector systems

    NASA Technical Reports Server (NTRS)

    Meegan, C. A.

    1981-01-01

    The performance of photomultiplier tubes (PMT's) and scintillation detector systems incorporating 50.8 by 1.27 cm NaI (T l) crystals was investigated to determine the characteristics of the photomultiplier tubes and optimize the detector geometry for the Burst and Transient Source Experiment on the Gamma Ray Observatory. Background information on performance characteristics of PMT's and NaI (T l) detectors is provided, procedures for measurement of relevant parameters are specified, and results of these measurements are presented.

  10. Fundamental Limits of Scintillation Detector Timing Precision

    PubMed Central

    Derenzo, Stephen E.; Choong, Woon-Seng; Moses, William W.

    2014-01-01

    In this paper we review the primary factors that affect the timing precision of a scintillation detector. Monte Carlo calculations were performed to explore the dependence of the timing precision on the number of photoelectrons, the scintillator decay and rise times, the depth of interaction uncertainty, the time dispersion of the optical photons (modeled as an exponential decay), the photodetector rise time and transit time jitter, the leading-edge trigger level, and electronic noise. The Monte Carlo code was used to estimate the practical limits on the timing precision for an energy deposition of 511 keV in 3 mm × 3 mm × 30 mm Lu2SiO5:Ce and LaBr3:Ce crystals. The calculated timing precisions are consistent with the best experimental literature values. We then calculated the timing precision for 820 cases that sampled scintillator rise times from 0 to 1.0 ns, photon dispersion times from 0 to 0.2 ns, photodetector time jitters from 0 to 0.5 ns fwhm, and A from 10 to 10,000 photoelectrons per ns decay time. Since the timing precision R was found to depend on A−1/2 more than any other factor, we tabulated the parameter B, where R = BA−1/2. An empirical analytical formula was found that fit the tabulated values of B with an rms deviation of 2.2% of the value of B. The theoretical lower bound of the timing precision was calculated for the example of 0.5 ns rise time, 0.1 ns photon dispersion, and 0.2 ns fwhm photodetector time jitter. The lower bound was at most 15% lower than leading-edge timing discrimination for A from 10 to 10,000 photoelectrons/ns. A timing precision of 8 ps fwhm should be possible for an energy deposition of 511 keV using currently available photodetectors if a theoretically possible scintillator were developed that could produce 10,000 photoelectrons/ns. PMID:24874216

  11. First-principles Electronic Structure Calculations for Scintillation Phosphor Nuclear Detector Materials

    NASA Astrophysics Data System (ADS)

    Canning, Andrew

    2013-03-01

    Inorganic scintillation phosphors (scintillators) are extensively employed as radiation detector materials in many fields of applied and fundamental research such as medical imaging, high energy physics, astrophysics, oil exploration and nuclear materials detection for homeland security and other applications. The ideal scintillator for gamma ray detection must have exceptional performance in terms of stopping power, luminosity, proportionality, speed, and cost. Recently, trivalent lanthanide dopants such as Ce and Eu have received greater attention for fast and bright scintillators as the optical 5d to 4f transition is relatively fast. However, crystal growth and production costs remain challenging for these new materials so there is still a need for new higher performing scintillators that meet the needs of the different application areas. First principles calculations can provide a useful insight into the chemical and electronic properties of such materials and hence can aid in the search for better new scintillators. In the past there has been little first-principles work done on scintillator materials in part because it means modeling f electrons in lanthanides as well as complex excited state and scattering processes. In this talk I will give an overview of the scintillation process and show how first-principles calculations can be applied to such systems to gain a better understanding of the physics involved. I will also present work on a high-throughput first principles approach to select new scintillator materials for fabrication as well as present more detailed calculations to study trapping process etc. that can limit their brightness. This work in collaboration with experimental groups has lead to the discovery of some new bright scintillators. Work supported by the U.S. Department of Homeland Security and carried out under U.S. Department of Energy Contract no. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory.

  12. Molecular origins of scintillation in organic scintillators (Conference Presentation)

    NASA Astrophysics Data System (ADS)

    Feng, Patrick; Mengesha, Wondwosen; Myllenbeck, Nicholas

    2016-09-01

    Organic-based scintillators are indispensable materials for radiation detection owing to their high sensitivity to fast neutrons, low cost, and tailorable properties. There has been a recent resurgence of interest in organic scintillators due to exciting discoveries related to neutron discrimination and gamma-ray spectroscopy, which represent capabilities previously thought not possible in these materials. I will discuss our development of crystalline and polymer-based scintillators for these applications. Structure-property relationships related to intermolecular interactions and host-guest electronic exchange will be discussed in the context of energy-transfer pathways relevant to scintillation. An emphasis will be placed on the rational design of these materials, as guided by first principles and DFT calculations. Two related topics will be discussed: 1) Incorporation of organometallic triplet-harvesting additives to plastic scintillator matrices to confer a 'two-state' (singlet and triplet) luminescence signature to different types of ionizing radiation. This approach relies upon energetic and spatial overlap between the donor and acceptor excited states for efficient electronic exchange. Key considerations also include synthetic modification of the luminescence spectra and kinetics, as well as the addition of secondary additives to increase the recombination efficiency. 2) Design of organotin-containing plastic scintillators as a route towards gamma-ray spectroscopy. Organometallic compounds were selected on the basis of distance-dependent quenching relationships, phase compatibility with the polymer matrix, and the gamma-ray cross sections. This approach is guided by molecular modeling and radiation transport modeling to achieve the highest possible detection sensitivity luminescence intensity.

  13. FNAL-NICADD extruded scintillator

    SciTech Connect

    Beznosko, D.; Bross, A.; Dyshkant, A.; Pla-Dalmau, A.; Rykalin, V.; /Northern Illinois U.

    2005-09-01

    The possibility to produce a scintillator that satisfies the demands of physicists from different science areas has emerged with the installation of an extrusion line at Fermi National Accelerator Laboratory (FNAL). The extruder is the product of the fruitful collaboration between FNAL and Northern Illinois Center for Accelerator and Detector Development (NICADD) at Northern Illinois University (NIU). The results from the light output, light attenuation length and mechanical tolerance indicate that FNAL-NICADD scintillator is of high quality. Improvements in the extrusion die will yield better scintillator profiles and decrease the time needed for initial tuning. This paper will present the characteristics of the FNAL-NICADD scintillator based on the measurements performed. They include the response to MIPs from cosmic rays for individual extruded strips and irradiation studies where extruded samples were irradiated up to 1 Mrad. We will also discuss the results achieved with a new die design. The attractive perspective of using the extruded scintillator with MRS (Metal Resistive Semiconductor) photodetector readout will also be shown.

  14. Radiopure metal-loaded liquid scintillator

    SciTech Connect

    Rosero, Richard; Yeh, Minfang

    2015-08-17

    Metal-loaded liquid scintillator plays a key role in particle and nuclear physics experiments. The applications of metal ions in various neutrino experiments and the purification methods for different scintillator components are discussed in this paper.

  15. Radiopure Metal-Loaded Liquid Scintillator

    SciTech Connect

    Rosero, Richard; Yeh, Minfang

    2015-03-18

    Metal-loaded liquid scintillator plays a key role in particle and nuclear physics experiments. The applications of metal ions in various neutrino experiments and the purification methods for different scintillator components are discussed in this paper.

  16. Advances in scintillators for medical imaging applications

    NASA Astrophysics Data System (ADS)

    van Loef, Edgar V.; Shah, Kanai S.

    2014-09-01

    A review is presented of some recent work in the field of inorganic scintillator research for medical imaging applications, in particular scintillation detectors for Single-Photon Emission Computed Tomography (SPECT) and Positron Emission Tomography (PET).

  17. Scintillating glass fiber neutron senors

    SciTech Connect

    Abel, K.H.; Arthur, R.J.; Bliss, M.

    1994-04-01

    Cerium-doped lithium-silicate glass fibers have been developed at Pacific Northwest Laboratory (PNL) for use as thermal neutron detectors. By using highly-enriched {sup 6} Li , these fibers efficiently capture thermal neutrons and produce scintillation light that can be detected at the ends of the fibers. Advantages of scintillating fibers over {sup 3}He or BF{sub 3} proportional tubes include flexibility in geometric configuration, ruggedness in high-vibration environments, and less detector weight for the same neutron sensitivity. This paper describes the performance of these scintillating fibers with regard to count rates, pulse height spectra, absolute efficiencies, and neutron/gamma discrimination. Fibers with light transmission lengths (1/e) of greater than 2 m have been produced at PNL. Neutron sensors in fiber form allow development of a variety of neutron detectors packaged in previously unavailable configurations. Brief descriptions of some of the devices already produced are included to illustrate these possibilities.

  18. Scintillation-Hardened GPS Receiver

    NASA Technical Reports Server (NTRS)

    Stephens, Donald R.

    2015-01-01

    CommLargo, Inc., has developed a scintillation-hardened Global Positioning System (GPS) receiver that improves reliability for low-orbit missions and complies with NASA's Space Telecommunications Radio System (STRS) architecture standards. A software-defined radio (SDR) implementation allows a single hardware element to function as either a conventional radio or as a GPS receiver, providing backup and redundancy for platforms such as the International Space Station (ISS) and high-value remote sensing platforms. The innovation's flexible SDR implementation reduces cost, weight, and power requirements. Scintillation hardening improves mission reliability and variability. In Phase I, CommLargo refactored an open-source GPS software package with Kalman filter-based tracking loops to improve performance during scintillation and also demonstrated improved navigation during a geomagnetic storm. In Phase II, the company generated a new field-programmable gate array (FPGA)-based GPS waveform to demonstrate on NASA's Space Communication and Navigation (SCaN) test bed.

  19. Liquid scintillator tiles for calorimetry

    DOE PAGES

    Amouzegar, M.; Belloni, A.; Bilki, B.; ...

    2016-11-28

    Future experiments in high energy and nuclear physics may require large, inexpensive calorimeters that can continue to operate after receiving doses of 50 Mrad or more. Also, the light output of liquid scintillators suffers little degradation under irradiation. However, many challenges exist before liquids can be used in sampling calorimetry, especially regarding developing a packaging that has sufficient efficiency and uniformity of light collection, as well as suitable mechanical properties. We present the results of a study of a scintillator tile based on the EJ-309 liquid scintillator using cosmic rays and test beam on the light collection efficiency and uniformity,more » and some preliminary results on radiation hardness.« less

  20. Unitary scintillation detector and system

    DOEpatents

    McElhaney, Stephanie A.; Chiles, Marion M.

    1994-01-01

    The invention is a unitary alpha, beta, and gamma scintillation detector and system for sensing the presence of alpha, beta, and gamma radiations selectively or simultaneously. The scintillators are mounted in a light-tight housing provided with an entrance window for admitting alpha, beta, and gamma radiation and excluding ambient light from the housing. Light pulses from each scintillator have different decay constants that are converted by a photosensitive device into corresponding differently shaped electrical pulses. A pulse discrimination system identifies the electrical pulses by their respective pulse shapes which are determined by decay time. The identified electrical pulses are counted in separate channel analyzers to indicate the respective levels of sensed alpha, beta, and gamma radiations.

  1. Unitary scintillation detector and system

    DOEpatents

    McElhaney, S.A.; Chiles, M.M.

    1994-05-31

    The invention is a unitary alpha, beta, and gamma scintillation detector and system for sensing the presence of alpha, beta, and gamma radiations selectively or simultaneously. The scintillators are mounted in a light-tight housing provided with an entrance window for admitting alpha, beta, and gamma radiation and excluding ambient light from the housing. Light pulses from each scintillator have different decay constants that are converted by a photosensitive device into corresponding differently shaped electrical pulses. A pulse discrimination system identifies the electrical pulses by their respective pulse shapes which are determined by decay time. The identified electrical pulses are counted in separate channel analyzers to indicate the respective levels of sensed alpha, beta, and gamma radiations. 10 figs.

  2. Development of radiation hard scintillators

    SciTech Connect

    Markley, F.; Woods, D.; Pla-Dalmau, A.; Foster, G. ); Blackburn, R. )

    1992-05-01

    Substantial improvements have been made in the radiation hardness of plastic scintillators. Cylinders of scintillating materials 2.2 cm in diameter and 1 cm thick have been exposed to 10 Mrads of gamma rays at a dose rate of 1 Mrad/h in a nitrogen atmosphere. One of the formulations tested showed an immediate decrease in pulse height of only 4% and has remained stable for 12 days while annealing in air. By comparison a commercial PVT scintillator showed an immediate decrease of 58% and after 43 days of annealing in air it improved to a 14% loss. The formulated sample consisted of 70 parts by weight of Dow polystyrene, 30 pbw of pentaphenyltrimethyltrisiloxane (Dow Corning DC 705 oil), 2 pbw of p-terphenyl, 0.2 pbw of tetraphenylbutadiene, and 0.5 pbw of UVASIL299LM from Ferro.

  3. Nanophosphor composite scintillator with a liquid matrix

    DOEpatents

    McKigney, Edward Allen; Burrell, Anthony Keiran; Bennett, Bryan L.; Cooke, David Wayne; Ott, Kevin Curtis; Bacrania, Minesh Kantilal; Del Sesto, Rico Emilio; Gilbertson, Robert David; Muenchausen, Ross Edward; McCleskey, Thomas Mark

    2010-03-16

    An improved nanophosphor scintillator liquid comprises nanophosphor particles in a liquid matrix. The nanophosphor particles are optionally surface modified with an organic ligand. The surface modified nanophosphor particle is essentially surface charge neutral, thereby preventing agglomeration of the nanophosphor particles during dispersion in a liquid scintillator matrix. The improved nanophosphor scintillator liquid may be used in any conventional liquid scintillator application, including in a radiation detector.

  4. Characteristics of Un doped and Europium-dopedSrI2 Scintillator Detectors

    SciTech Connect

    Sturm, Benjamin; Cherepy, Nerine; Drury, Owen; Thelin, P; Fisher, S E; O’Neal, S P; Payne, Stephen A.; Burger, Arnold; Boatner, Lynn A; Ramey, Joanne Oxendine; Shah, Kanai; Hawrami, Rastgo

    2012-01-01

    High energy resolution gamma-ray detectors that can be formed into relatively large sizes while operating at room temperature offer many advantages for national security applications. We are working toward that goal through the development of SrI{sub 2}(Eu) scintillator detectors, which routinely provide <;3.0% energy resolution at 662 keV with volumes >;10 cm{sup 3}. In this study, we have tested pure, undoped SrI{sub 2} to gain a better understanding of the scintillation properties and spectroscopic performance achievable without activation. An undoped crystal grown from 99.999% pure SrI{sub 2} pellets was tested for its spectroscopic performance, its light yield, and uniformity of scintillation light collection as a function of gamma-ray interaction position relative to the crystal growth direction. Undoped SrI{sub 2} was found to provide energy resolution of 5.3% at 662 keV, and the light collection nonuniformity varied by only 0.72% over the length of the crystal. Measurements of both a 3% Eu-doped and the undoped SrI{sub 2} crystal were carried out in the SLYNCI facility and indicate differences in their light yield non-proportionality. The surprisingly good scintillation properties of the pure SrI{sub 2} crystal suggests that with high-purity feedstock, further reduction of the Eu concentration can be made to grow larger crystals while not adversely impacting the spectroscopic performance.

  5. An active electron polarized scintillating GSO target for neutrino physics

    NASA Astrophysics Data System (ADS)

    Baiboussinov, B.; Braggio, C.; Cardini, A.; Carugno, G.; Congiu, F.; Gain, S.; Galeazzi, G.; Lai, A.; Lehman, A.; Mocci, P.; Mura, A.; Quochi, F.; Saba, M.; Saitta, B.; Sartori, G.

    2012-12-01

    The feasibility of an electron-polarized, active target to be used as detector in neutrino scattering experiments, suggested by several theoretical papers, has been investigated. We report on the properties of the paramagnetic crystal Gd2SiO5 (GSO), in which 7.7% of the total number of electrons present can be polarized by lowering the temperature and applying an intense external magnetic field. The material magnetic susceptibility has been measured down to cryogenic temperatures showing that for H=5 T and T=4 K about 80% of the maximum allowed magnetization can be attained. Also the spectral and time response of the crystal have been characterized and the scintillation process has been studied using a photomultiplier to measure the response to gamma rays irradiation and cosmic rays operating the GSO crystal at 13.5 K. An avalanche photodiode (APD) readout of the scintillation signal from the GSO crystal has also been performed, since the magnetic field-independent response of this device allows it to be placed close to the crystal in the cryogenic environment.

  6. Characteristics of High Latitude Ionosphere Scintillations

    NASA Astrophysics Data System (ADS)

    Morton, Y.

    2012-12-01

    As we enter a new solar maximum period, global navigation satellite systems (GNSS) receivers, especially the ones operating in high latitude and equatorial regions, are facing an increasing threat from ionosphere scintillations. The increased solar activities, however, also offer a great opportunity to collect scintillation data to characterize scintillation signal parameters and ionosphere irregularities. While there are numerous GPS receivers deployed around the globe to monitor ionosphere scintillations, most of them are commercial receivers whose signal processing mechanisms are not designed to operate under ionosphere scintillation. As a result, they may distort scintillation signal parameters or lose lock of satellite signals under strong scintillations. Since 2008, we have established and continuously improved a unique GNSS receiver array at HAARP, Alaska. The array contains high ends commercial receivers and custom RF front ends which can be automatically triggered to collect high quality GPS and GLONASS satellite signals during controlled heating experiments and natural scintillation events. Custom designed receiver signal tracking algorithms aim to preserve true scintillation signatures are used to process the raw RF samples. Signal strength, carrier phase, and relative TEC measurements generated by the receiver array since its inception have been analyzed to characterize high latitude scintillation phenomena. Daily, seasonal, and solar events dependency of scintillation occurrence, spectral contents of scintillation activities, and plasma drifts derived from these measurements will be presented. These interesting results demonstrate the feasibility and effectiveness of our experimental data collection system in providing insightful details of ionosphere responses to active perturbations and natural disturbances.

  7. Composite scintillators for detection of ionizing radiation

    DOEpatents

    Dai, Sheng [Knoxville, TN; Stephan, Andrew Curtis [Knoxville, TN; Brown, Suree S [Knoxville, TN; Wallace, Steven A [Knoxville, TN; Rondinone, Adam J [Knoxville, TN

    2010-12-28

    Applicant's present invention is a composite scintillator having enhanced transparency for detecting ionizing radiation comprising a material having optical transparency wherein said material comprises nano-sized objects having a size in at least one dimension that is less than the wavelength of light emitted by the composite scintillator wherein the composite scintillator is designed to have selected properties suitable for a particular application.

  8. Optical simulation of monolithic scintillator detectors using GATE/GEANT4.

    PubMed

    van der Laan, D J Jan; Schaart, Dennis R; Maas, Marnix C; Beekman, Freek J; Bruyndonckx, Peter; van Eijk, Carel W E

    2010-03-21

    Much research is being conducted on position-sensitive scintillation detectors for medical imaging, particularly for emission tomography. Monte Carlo simulations play an essential role in many of these research activities. As the scintillation process, the transport of scintillation photons through the crystal(s), and the conversion of these photons into electronic signals each have a major influence on the detector performance; all of these processes may need to be incorporated in the model to obtain accurate results. In this work the optical and scintillation models of the GEANT4 simulation toolkit are validated by comparing simulations and measurements on monolithic scintillator detectors for high-resolution positron emission tomography (PET). We have furthermore made the GEANT4 optical models available within the user-friendly GATE simulation platform (as of version 3.0). It is shown how the necessary optical input parameters can be determined with sufficient accuracy. The results show that the optical physics models of GATE/GEANT4 enable accurate prediction of the spatial and energy resolution of monolithic scintillator PET detectors.

  9. Synthesis of plastic scintillation microspheres: Evaluation of scintillators

    NASA Astrophysics Data System (ADS)

    Santiago, L. M.; Bagán, H.; Tarancón, A.; Garcia, J. F.

    2013-01-01

    The use of plastic scintillation microspheres (PSm) appear to be an alternative to liquid scintillation for the quantification of alpha and beta emitters because it does not generate mixed wastes after the measurement (organic and radioactive). In addition to routine radionuclide determinations, PSm can be used for further applications, e.g. for usage in a continuous monitoring equipment, for measurements of samples with a high salt concentration and for an extractive scintillation support which permits the separation, pre-concentration and measurement of the radionuclides without additional steps of elution and sample preparation. However, only a few manufacturers provide PSm, and the low number of regular suppliers reduces its availability and restricts the compositions and sizes available. In this article, a synthesis method based on the extraction/evaporation methodology has been developed and successfully used for the synthesis of plastic scintillation microspheres. Seven different compositions of plastic scintillation microspheres have been synthesised; PSm1 with polystyrene, PSm2 with 2,5-Diphenyloxazol(PPO), PSm3 with p-terphenyl (pT), PSm4 with PPO and 1,4-bis(5-phenyloxazol-2-yl) (POPOP), PSm5 pT and (1,4-bis [2-methylstyryl] benzene) (Bis-MSB), PSm6 with PPO, POPOP and naphthalene and PSm7 with pT, Bis-MSB and naphthalene. The synthesised plastic scintillation microspheres have been characterised in terms of their morphology, detection capabilities and alpha/beta separation capacity. The microspheres had a median diameter of approximately 130 μm. Maximum detection efficiency values were obtained for the PSm4 composition as follows 1.18% for 3H, 51.2% for 14C, 180.6% for 90Sr/90Y and 76.7% for 241Am. Values of the SQP(E) parameter were approximately 790 for PSm4 and PSm5. These values show that the synthesised PSm exhibit good scintillation properties and that the spectra are at channel numbers higher than in commercial PSm. Finally, the addition of

  10. Rejection of Alpha Surface Background in Non-scintillating Bolometric Detectors: The ABSuRD Project

    NASA Astrophysics Data System (ADS)

    Biassoni, M.; Brofferio, C.; Bucci, C.; Canonica, L.; di Vacri, M. L.; Gorla, P.; Pavan, M.; Yeh, M.

    2016-08-01

    Due to their excellent energy resolution values and the vast choice of possible materials, bolometric detectors are currently widely used in the physics of rare events. A limiting aspect for bolometers rises from their inability to discriminate among radiation types or surface from bulk events. It has been demonstrated that the main limitation to sensitivity for purely bolometric detectors is represented by surface alpha contaminations, causing a continuous background that cannot be discriminated. A new scintillation-based technique for the rejection of surface alpha background in non-scintillating bolometric experiments is proposed in this work. The idea is to combine a scintillating and a high sensitivity photon detector with a non-scintillating absorber. We present results showing the possibility to reject events due to alpha decay at or nearby the surface of the crystal.

  11. Rejection of Alpha Surface Background in Non-scintillating Bolometric Detectors: The ABSuRD Project

    SciTech Connect

    Biassoni, M.; Brofferio, C.; Bucci, C.; Canonica, L.; di Vacri, M. L.; Gorla, P.; Pavan, M.; Yeh, M.

    2016-01-14

    Due to their excellent energy resolution values and the vast choice of possible materials, bolometric detectors are currently widely used in the physics of rare events. A limiting aspect for bolometers rises from their inability to discriminate among radiation types or surface from bulk events. It has been demonstrated that the main limitation to sensitivity for purely bolometric detectors is represented by surface alpha contaminations, causing a continuous background that cannot be discriminated. A new scintillation based technique for the rejection of surface alpha background in non- scintillating bolometric experiments is proposed in this work. The idea is to combine a scintillating and a high sensitivity photon detector with a non- scintillating absorber. Finally, we present results showing the possibility to reject events due to alpha decay at or nearby the surface of the crystal.

  12. Rejection of Alpha Surface Background in Non-scintillating Bolometric Detectors: The ABSuRD Project

    DOE PAGES

    Biassoni, M.; Brofferio, C.; Bucci, C.; ...

    2016-01-14

    Due to their excellent energy resolution values and the vast choice of possible materials, bolometric detectors are currently widely used in the physics of rare events. A limiting aspect for bolometers rises from their inability to discriminate among radiation types or surface from bulk events. It has been demonstrated that the main limitation to sensitivity for purely bolometric detectors is represented by surface alpha contaminations, causing a continuous background that cannot be discriminated. A new scintillation based technique for the rejection of surface alpha background in non- scintillating bolometric experiments is proposed in this work. The idea is to combinemore » a scintillating and a high sensitivity photon detector with a non- scintillating absorber. Finally, we present results showing the possibility to reject events due to alpha decay at or nearby the surface of the crystal.« less

  13. Melt-cast organic glasses as high-efficiency fast neutron scintillators

    DOE PAGES

    Carlson, Joseph S.; Feng, Patrick L.

    2016-06-24

    In this work we report a new class of organic-based scintillators that combines several of the desirable attributes of existing crystalline, liquid, and plastic organic scintillators. The prepared materials may be isolated in single crystalline form or melt-cast to produce highly transparent glasses that have been shown to provide high light yields of up to 16,000 photons/MeVee, as evaluated against EJ-200 plastic scintillators and solution-grown trans-stilbene crystals. The prepared organic glasses exhibit neutron/gamma pulse-shape discrimination (PSD) and are compatible with wavelength shifters to reduce optical self-absorption effects that are intrinsic to pure materials such as crystalline organics. In conclusion, themore » combination of high scintillation efficiency, PSD capabilities, and facile scale-up via melt-casting distinguishes this new class of amorphous materials from existing alternatives.« less

  14. Melt-cast organic glasses as high-efficiency fast neutron scintillators

    SciTech Connect

    Carlson, Joseph S.; Feng, Patrick L.

    2016-06-24

    In this work we report a new class of organic-based scintillators that combines several of the desirable attributes of existing crystalline, liquid, and plastic organic scintillators. The prepared materials may be isolated in single crystalline form or melt-cast to produce highly transparent glasses that have been shown to provide high light yields of up to 16,000 photons/MeVee, as evaluated against EJ-200 plastic scintillators and solution-grown trans-stilbene crystals. The prepared organic glasses exhibit neutron/gamma pulse-shape discrimination (PSD) and are compatible with wavelength shifters to reduce optical self-absorption effects that are intrinsic to pure materials such as crystalline organics. In conclusion, the combination of high scintillation efficiency, PSD capabilities, and facile scale-up via melt-casting distinguishes this new class of amorphous materials from existing alternatives.

  15. New detecting techniques for a future calorimetry

    NASA Astrophysics Data System (ADS)

    Auffray, E.; Buganov, O.; Fedorov, A.; Korjik, M.; Lecoq, P.; Tamulaitis, G.; Tikhomirov, S.; Vasil'ev, A.

    2015-02-01

    In the last forty years, application of crystalline materials in homogeneous Electromagnetic Calorimeters has played a crucial role in the discovery of matter properties and promoted a continuous progress in the detecting technique. The detection systems progressed from small detectors based on NaI(Tl), CsI(Na), BaF2, PbF2, and Bi4Ge3O12 to giant Electromagnetic Calorimeters of CMS, ALICE Collaborations at LHC and PANDA Collaboration at FAIR, where the systems consisted of thousands lead tungstate PbWO4 scintillation crystals. Lead tungstate (PWO) became the most extensively used scintillation material in high energy physics experiments. PWO possesses a unique combination of scintillation properties including high energy and time resolutions in the detection of high energy particles. Here, we report on the results of the two photon absorption in PWO crystals obtained by pump-probe technique using ultra short laser pulses. The results demonstrate that the relaxation processes in PWO offer capability of this material to be used in detection systems to make a time stamp with precision close to 10-12 s or even better.

  16. Chloride, bromide and iodide scintillators with europium doping

    DOEpatents

    Zhuravleva, Mariya; Yang, Kan

    2014-08-26

    A halide scintillator material is disclosed where the halide may comprise chloride, bromide or iodide. The material is single-crystalline and has a composition of the general formula ABX.sub.3 where A is an alkali, B is an alkali earth and X is a halide which general composition was investigated. In particular, crystals of the formula ACa.sub.1-yEu.sub.yI.sub.3 where A=K, Rb and Cs were formed as well as crystals of the formula CsA.sub.1-yEu.sub.yX.sub.3 (where A=Ca, Sr, Ba, or a combination thereof and X=Cl, Br or I or a combination thereof) with divalent Europium doping where 0.ltoreq.y.ltoreq.1, and more particularly Eu doping has been studied at one to ten mol %. The disclosed scintillator materials are suitable for making scintillation detectors used in applications such as medical imaging and homeland security.

  17. Extruded plastic scintillator for MINERvA

    SciTech Connect

    Pla-Dalmau, Anna; Bross, Alan D.; Rykalin, Victor V.; Wood, Brian M.; /NICADD, DeKalb

    2005-11-01

    An extrusion line has recently been installed at Fermilab in collaboration with NICADD (Northern Illinois Center for Accelerator and Detector Development). This new facility will serve to further develop and improve extruded plastic scintillator. Since polystyrene is widely used in the consumer industry, the logical path was to investigate the extrusion of commercial-grade polystyrene pellets with dopants to yield high quality plastic scintillator. The D0 and MINOS experiments are already using extruded scintillator strips in their detectors. A new experiment at Fermilab is pursuing the use of extruded plastic scintillator. A new plastic scintillator strip is being tested and its properties characterized. The initial results are presented here.

  18. SNO+ Scintillator Purification and Assay

    SciTech Connect

    Ford, R.; Vazquez-Jauregui, E.; Chen, M.; Chkvorets, O.; Hallman, D.

    2011-04-27

    We describe the R and D on the scintillator purification and assay methods and technology for the SNO+ neutrino and double-beta decay experiment. The SNO+ experiment is a replacement of the SNO heavy water with liquid scintillator comprised of 2 g/L PPO in linear alkylbenzene (LAB). During filling the LAB will be transported underground by rail car and purified by multi-stage distillation and steam stripping at a flow rate of 19 LPM. While the detector is operational the scintillator can be recirculated at 150 LPM (full detector volume in 4 days) to provide repurification as necessary by either water extraction (for Ra, K, Bi) or by functional metal scavenger columns (for Pb, Ra, Bi, Ac, Th) followed by steam stripping to remove noble gases and oxygen (Rn, O{sub 2}, Kr, Ar). The metal scavenger columns also provide a method for scintillator assay for ex-situ measurement of the U and Th chain radioactivity. We have developed ''natural'' radioactive spikes of Pb and Ra in LAB and use these for purification testing. Lastly, we present the planned operating modes and purification strategies and the plant specifications and design.

  19. SNO+ Scintillator Purification and Assay

    NASA Astrophysics Data System (ADS)

    Ford, R.; Chen, M.; Chkvorets, O.; Hallman, D.; Vázquez-Jáuregui, E.

    2011-04-01

    We describe the R&D on the scintillator purification and assay methods and technology for the SNO+ neutrino and double-beta decay experiment. The SNO+ experiment is a replacement of the SNO heavy water with liquid scintillator comprised of 2 g/L PPO in linear alkylbenzene (LAB). During filling the LAB will be transported underground by rail car and purified by multi-stage distillation and steam stripping at a flow rate of 19 LPM. While the detector is operational the scintillator can be recirculated at 150 LPM (full detector volume in 4 days) to provide repurification as necessary by either water extraction (for Ra, K, Bi) or by functional metal scavenger columns (for Pb, Ra, Bi, Ac, Th) followed by steam stripping to remove noble gases and oxygen (Rn, O2, Kr, Ar). The metal scavenger columns also provide a method for scintillator assay for ex-situ measurement of the U and Th chain radioactivity. We have developed "natural" radioactive spikes of Pb and Ra in LAB and use these for purification testing. Lastly, we present the planned operating modes and purification strategies and the plant specifications and design.

  20. Maximum likelihood positioning and energy correction for scintillation detectors

    NASA Astrophysics Data System (ADS)

    Lerche, Christoph W.; Salomon, André; Goldschmidt, Benjamin; Lodomez, Sarah; Weissler, Björn; Solf, Torsten

    2016-02-01

    An algorithm for determining the crystal pixel and the gamma ray energy with scintillation detectors for PET is presented. The algorithm uses Likelihood Maximisation (ML) and therefore is inherently robust to missing data caused by defect or paralysed photo detector pixels. We tested the algorithm on a highly integrated MRI compatible small animal PET insert. The scintillation detector blocks of the PET gantry were built with the newly developed digital Silicon Photomultiplier (SiPM) technology from Philips Digital Photon Counting and LYSO pixel arrays with a pitch of 1 mm and length of 12 mm. Light sharing was used to readout the scintillation light from the 30× 30 scintillator pixel array with an 8× 8 SiPM array. For the performance evaluation of the proposed algorithm, we measured the scanner’s spatial resolution, energy resolution, singles and prompt count rate performance, and image noise. These values were compared to corresponding values obtained with Center of Gravity (CoG) based positioning methods for different scintillation light trigger thresholds and also for different energy windows. While all positioning algorithms showed similar spatial resolution, a clear advantage for the ML method was observed when comparing the PET scanner’s overall single and prompt detection efficiency, image noise, and energy resolution to the CoG based methods. Further, ML positioning reduces the dependence of image quality on scanner configuration parameters and was the only method that allowed achieving highest energy resolution, count rate performance and spatial resolution at the same time.

  1. FLARES: A flexible scintillation light apparatus for rare event searches

    NASA Astrophysics Data System (ADS)

    Sisti, M.; Baldazzi, G.; Bonvicini, V.; Campana, R.; Capelli, S.; Evangelista, Y.; Feroci, M.; Fuschino, F.; Gironi, L.; Labanti, C.; Marisaldi, M.; Previtali, E.; Rignanese, L.; Rachevsky, A.; Vacchi, A.; Zampa, G.; Zampa, N.; Zuffa, M.

    2016-07-01

    FLARES is a project for an innovative detector technology to be applied to rare event searches, and in particular to neutrinoless double beta decay experiments. Its novelty is the enhancement and optimization of the collection of the scintillation light emitted by ultra-pure crystals through the use of arrays of high performance silicon photodetectors cooled to 120 K. This would provide scintillation detectors with 1% level energy resolution, with the advantages of a technology offering relatively simple low cost mass scalability and powerful background reduction handles, as requested by future neutrinoless double beta decay experimental programs. The performances of a first production of matrices of Silicon Drift Detectors are presented and discussed in this paper.

  2. An apparatus for studying scintillator properties at high isostatic pressures

    SciTech Connect

    Gaume, R. M.; Lam, S.; Gascon, M.; Feigelson, R. S.; Setyawan, W.; Curtarolo, S.

    2013-01-15

    We describe the design and operation of a unique hydraulic press for the study of scintillator materials under isostatic pressure. This press, capable of developing a pressure of a gigapascal, consists of a large sample chamber pressurized by a two-stage hydraulic amplifier. The optical detection of the scintillation light emitted by the sample is performed, through a large aperture optical port, by a photodetector located outside the pressure vessel. In addition to providing essential pressure-dependent studies on the emission characteristics of radioluminescent materials, this apparatus is being developed to elucidate the mechanisms behind the recently observed dependency of light-yield nonproportionality on electronic band structure. The variation of the light output of a Tl:CsI crystal under 511-keV gamma excitation and hydrostatic pressure is given as an example.

  3. Mercuric Iodide Photocell Technology for Room Temperature Readout of Scintillators

    SciTech Connect

    Warnick Kernan et al.

    2007-08-31

    Mercuric iodide (HgI2) is a well known material for the direct detection of gamma rays; however, the largest volume achievable is limited by thickness of the detector, which needs to be a small fraction of the average trapping length for electrons. We are reporting here preliminary results in using HgI2 crystals to fabricate photocells used in the readout of various scintillators. The optical spectral response and efficiency of these photocells were measured and will be reported. Preliminary nuclear response from a HgI2 photocell that was optically matched to a Ce3+ :LaBr3 scintillator will also be presented and discussed. Further improvements will be sought by optimizing the transparent contact technology.

  4. Scintillation properties of LuI 3:Ce

    NASA Astrophysics Data System (ADS)

    Glodo, J.; Shah, K. S.; Klugerman, M.; Wong, P.; Higgins, B.; Dorenbos, P.

    2005-01-01

    Lutetium iodide (LuI3) is a new addition to the family of Ce-doped lanthanide trihalide scintillating materials. Crystals of this material show hexagonal structure with density of 5.6 g/cm3 and have been grown by the Bridgman method. Under X-ray excitation this material exhibits broad, cerium based emission that peaks at 475 and 520 nm. The fastest and major component of scintillation time profile of LuI3:Ce emission decays with a 31 ns time constant. The light yield of LuI3:Ce for thin samples (∼0.2 mm) was estimated to be ∼50,000 photons/MeV.

  5. Precision Crystal Calorimeters in High Energy Physics

    ScienceCinema

    Ren-Yuan Zhu

    2016-07-12

    Precision crystal calorimeters traditionally play an important role in high energy physics experiments. In the last two decades, it faces a challenge to maintain its precision in a hostile radiation environment. This paper reviews the performance of crystal calorimeters constructed for high energy physics experiments and the progress achieved in understanding crystal’s radiation damage as well as in developing high quality scintillating crystals for particle physics. Potential applications of new generation scintillating crystals of high density and high light yield, such as LSO and LYSO, in particle physics experiments is also discussed.

  6. LiCaAlF6 scintillators in neutron and gamma radiation fields

    NASA Astrophysics Data System (ADS)

    Viererbl, L.; Klupák, V.; Vinš, M.; Koleška, M.; Šoltés, J.; Yoshikawa, A.; Nikl, M.

    2016-09-01

    Intentionally doped LiCaAlF6 (LiCAF) single crystals are prospective scintillators, especially for thermal neutron detection through the 6Li(n,t)4He nuclear reaction. Four different LiCAF scintillator samples were tested in various neutron and gamma fields. Two of the tested samples were LiCAF:Eu and LiCAF:Eu,Na single crystals, and another two samples were made of LiCAF:Eu micro crystals dispersed in transparent rubber, with different rubber dimensions. All LiCAF samples contain lithium enriched to6Li. A plutonium-beryllium source was used as a neutron source. The neutron spectrum was modified by moderator and filter to get different ratios between thermal, epithermal and fast neutron fluence rates. The MCNP code was used for calculations of the fluence rates for different configurations. Radionuclides 137Cs and 60Co were applied as gamma radiation sources. The light signal from the scintillator was evaluated with a photomultiplier and a multichannel analyzer. The purpose of this work was to study the characteristics of LiCAF scintillators, especially the ability to discriminate signals from neutron and gamma radiation, which is the basic scintillator condition for neutron detection in mixed neutron-gamma radiation fields. Generally, the discrimination can be done by the pulse height and/or the pulse shape of the evaluated signals. Both methods can be used for a LiCAF scintillator. However, only the pulse height discrimination method is discussed in this paper. The possibility of fast neutron detection with LiCAF scintillators was also tested.

  7. SrI2 scintillator for gamma ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Cherepy, N. J.; Sturm, B. W.; Drury, O. B.; Hurst, T. A.; Sheets, S. A.; Ahle, L. E.; Saw, C. K.; Pearson, M. A.; Payne, S. A.; Burger, A.; Boatner, L. A.; Ramey, J. O.; van Loef, E. V.; Glodo, J.; Hawrami, R.; Higgins, W. M.; Shah, K. S.; Moses, W. W.

    2009-08-01

    We are working to perfect the growth of divalent Eu-doped strontium iodide single crystals and to optimize the design of SrI2(Eu)-based gamma ray spectrometers. SrI2(Eu) offers a light yield in excess of 100,000 photons/MeV and light yield proportionality surpassing that of Ce-doped lanthanum bromide. Thermal and x-ray diffraction analyses of SrI2 and EuI2 indicate an excellent match in melting and crystallographic parameters, and very modest thermal expansion anisotropy. We have demonstrated energy resolution with SrI2(4-6%Eu) of 2.6% at 662 keV and 7.6% at 60 keV with small crystals, while the resolution degrades somewhat for larger sizes. Our experiments suggest that digital techniques may be useful in improving the energy resolution in large crystals impaired by light-trapping, in which scintillation light is re-absorbed and re-emitted in large and/or highly Eu2+ -doped crystals. The light yield proportionality of SrI2(Eu) is found to be superior to that of other known scintillator materials, such as LaBr3(Ce) and NaI(Tl).

  8. Scintillation properties of selected oxide monocrystals activated with Ce and Pr

    NASA Astrophysics Data System (ADS)

    Wojtowicz, Andrzej J.; Drozdowski, Winicjusz; Wisniewski, Dariusz; Lefaucheur, Jean-Luc; Galazka, Zbigniew; Gou, Zhenhui; Lukasiewicz, Tadeusz; Kisielewski, Jaroslaw

    2006-01-01

    In the last 10-15 years there has been a significant effort toward development of new, more efficient and faster materials for detection of ionizing radiation. A growing demand for better scintillator crystals for detection of 511 keV gamma particles has been due mostly to recent advances in modern imaging systems employing positron emitting radionuclides for medical diagnostics in neurology, oncology and cardiology. While older imaging systems were almost exclusively based on BGO and NaI:Tl crystals the new systems, e.g., ECAT Accel, developed by Siemens/CTI, are based on recently discovered and developed LSO (Lu 2SiO 5:Ce, Ce-activated lutetium oxyorthosilicate) crystals. Interestingly, despite very good properties of LSO, there still is a strong drive toward development of new scintillator crystals that would show even better performance and characteristics. In this presentation we shall review spectroscopic and scintillator characterization of new complex oxide crystals, namely LSO, LYSO, YAG, LuAP (LuAlO 3, lutetium aluminate perovskite) and LuYAP activated with Ce and Pr. The LSO:Ce crystals have been grown by CTI Inc (USA), LYSO:Ce, LuAP:Ce and LuYAP:Ce crystals have been grown by Photonic Materials Ltd., Scotland (PML is the only company providing large LuAP:Ce crystals on a commercial scale), while YAG:Pr and LuAP:Pr crystals have been grown by Institute of Electronic Materials Technology (Poland). All these crystals have been characterized at Institute of Physics, N. Copernicus University (Poland). We will review and compare results of measurements of radioluminescence, VUV spectroscopy, scintillation light yields, scintillation time profiles and low temperature thermoluminescence performed on these crystals. We will demonstrate that all experiments clearly indicate that there is a significant room for improvement of LuAP, LuYAP and YAG. While both Ce-activated LSO and LYSO perform very well, we also note that LuYAP:Ce, LuAP:Ce and YAG:Pr offer some

  9. The observation of scintillation in a hydrated inorganic compound: CeCl3 6H2O

    SciTech Connect

    Boatner, Lynn A; Neal, John S; Ramey, Joanne Oxendine; Chakoumakos, Bryan C; Custelcean, Radu

    2013-01-01

    We have recently reported the discovery of a new family of rare-earth metal-organic single-crystal scintillators based on Ce3+ as the activator ion. Starting with the CeCl3(CH3OH)4 prototype, this family of scintillators has recently been extended to include complex metal-organic adducts produced by reacting CeCl3 with heavier organics (e.g., isomers of propanol and butanol). Some of these new rare-earth metal-organic materials incorporated waters of hydration in their structures, and the observation of scintillation in these hydrated compounds was an original finding for any solid scintillator. In the present work, we now report what is apparently the initial observation of gamma-ray-excited scintillation in an inorganic hydrated material, namely single-crystal monoclinic CeCl3 6H2O. This observation shows that the mechanisms of the various scintillation energy-transfer processes are not blocked by the presence of waters of hydration in an inorganic material and that the observation of scintillation in other hydrated inorganic compounds is not precluded.

  10. The lower timing resolution bound for scintillators with non-negligible optical photon transport time in time-of-flight PET

    PubMed Central

    Vinke, Ruud; Olcott, Peter D.; Cates, Joshua W.; Levin, Craig S.

    2014-01-01

    In this work, a method is presented that can calculate the lower bound of the timing resolution for large scintillation crystals with non-negligible photon transport. Hereby, the timing resolution bound can directly be calculated from Monte Carlo generated arrival times of the scintillation photons. This method extends timing resolution bound calculations based on analytical equations, as crystal geometries can be evaluated that do not have closed form solutions of arrival time distributions. The timing resolution bounds are calculated for an exemplary 3 × 3 × 20 mm3 LYSO crystal geometry, with scintillation centers exponentially spread along the crystal length as well as with scintillation centers at fixed distances from the photosensor. Pulse shape simulations further show that analog photosensors intrinsically operate near the timing resolution bound, which can be attributed to the finite single photoelectron pulse rise time. PMID:25255807

  11. Comparative Gamma Spectroscopy with SrI2(Eu), GYGAG(Ce) and Bi-loaded Plastic Scintillators

    SciTech Connect

    Cherepy, Nerine; Payne, Stephen A.; Sturm, Benjamin; Kuntz, Joshua; Seeley, Zachary; Rupert, B. L.; Sanner, Robert; Drury, Owen; Hurst, T.; Fisher, S E; Groza, Michael; Matei, L.; Burger, Arnold; Hawrami, Rastgo; Shah, Kanai; Boatner, Lynn A

    2011-01-01

    We are developing new scintillator materials that offer potential for high resolution gamma ray spectroscopy at low cost. Single crystal SrI2(Eu) offers ~3% resolution at 662 keV, in sizes of ~1 in3. We have developed ceramics processing technology allowing us to achieve cubic inch scale transparent ceramic scintillators offering gamma spectroscopy performance superior to NaI(Tl). We fabricated a bismuth-loaded plastic scintillator that demonstrates energy resolution of ~8% at 662 keV in small sizes.

  12. Improved lithium iodide neutron scintillator with Eu2+ activation: The elimination of Suzuki-Phase precipitates

    DOE PAGES

    Boatner, Lynn A.; Comer, Eleanor P.; Wright, Gomez W.; ...

    2017-02-21

    Monovalent alkali halides such as NaI, CsI, and LiI are widely used as inorganic scintillators for radiation detection due to their light yield, the capability for the growth of large single crystals, relatively low cost, and other favorable characteristics. These materials are frequently activated through the addition of small amounts (e.g., a few hundred ppm) of elements such as thallium - or sodium in the case of CsI. The monovalent alkali halide scintillators can also be activated with low concentrations of Eu2+, however Eu activation has previously not been widely employed due to the non-uniform segregation of the divalent Eumore » dopant that leads to the formation of unwanted phases during Bridgman or other solidification crystal-growth methods. Specifically, for Eu concentrations near and above ~0.5%, Suzuki Phase precipitates form in the course of the melt-growth process, and these Suzuki Phase particles scatter the scintillation light. This adversely affects the scintillator performance via reduction in the optical transmission of the material, and depending on the crystal thickness and precipitated-particle concentration, this reduction can occur up to the point of opacity. Here we describe a post-growth process for the removal of Suzuki Phase precipitates from single crystals of the neutron scintillator LiI activated with Eu2+ at concentrations up to and in excess of 3 wt.%, and we correlate the resulting neutron-detection performance with the thermal processing methods used to remove the Suzuki Phase particles. Furthermore, the resulting improved scintillator properties using increased Eu activator levels are applicable to neutron imaging and active interrogation systems, and pulse-height gamma-ray spectroscopy rather than pulse-shape discrimination can be used to discriminate between gamma ray and neutron interaction events.« less

  13. LHCb Upgrade: Scintillating Fibre Tracker

    NASA Astrophysics Data System (ADS)

    Tobin, Mark

    2016-07-01

    The LHCb detector will be upgraded during the Long Shutdown 2 (LS2) of the LHC in order to cope with higher instantaneous luminosities and to read out the data at 40 MHz using a trigger-less read-out system. All front-end electronics will be replaced and several sub-detectors must be redesigned to cope with higher occupancy. The current tracking detectors downstream of the LHCb dipole magnet will be replaced by the Scintillating Fibre (SciFi) Tracker. The SciFi Tracker will use scintillating fibres read out by Silicon Photomultipliers (SiPMs). State-of-the-art multi-channel SiPM arrays are being developed to read out the fibres and a custom ASIC will be used to digitise the signals from the SiPMs. The evolution of the design since the Technical Design Report in 2014 and the latest R & D results are presented.

  14. Scintillation Monitoring Using Asymmetry Index

    NASA Astrophysics Data System (ADS)

    Shaikh, Muhammad Mubasshir; Mahrous, Ayman; Abdallah, Amr; Notarpietro, Riccardo

    Variation in electron density can have significant effect on GNSS signals in terms of propagation delay. Ionospheric scintillation can be caused by rapid change of such delay, specifically, when they last for a longer period of time. Ionospheric irregularities that account for scintillation may vary significantly in spatial range and drift with the background plasma at speeds of 45 to 130 m/sec. These patchy irregularities may occur several times during night, e.g. in equatorial region, with the patches move through the ray paths of the GNSS satellite signals. These irregularities are often characterized as either ‘large scale’ (which can be as large as several hundred km in East-West direction and many times that in the North-South direction) or ‘small scale’ (which can be as small as 1m). These small scale irregularities are regarded as the main cause of scintillation [1,2]. In normal solar activity conditions, the mid-latitude ionosphere is not much disturbed. However, during severe magnetic storms, the aurora oval extends towards the equator and the equator anomaly region may stretched towards poles extending the scintillation phenomena more typically associated with those regions into mid-latitudes. In such stormy conditions, the predicted TEC may deviate largely from the true value of the TEC both at low and mid-latitudes due to which GNSS applications may be strongly degraded. This work is an attempt to analyze ionospheric scintillation (S4 index) using ionospheric asymmetry index [3]. The asymmetry index is based on trans-ionospheric propagation between GPS and LEO satellites in a radio occultation (RO) scenario, using background ionospheric data provided by MIDAS [4]. We attempted to simulate one of the recent geomagnetic storms (NOAA scale G4) occurred over low/mid-latitudes. The storm started on 26 September 2011 at UT 18:00 and lasted until early hours of 27 September 2011. The scintillation data for the storm was taken from an ionospheric

  15. Detecting scintillations in liquid helium

    NASA Astrophysics Data System (ADS)

    Huffman, P. R.; McKinsey, D. N.

    2013-09-01

    We review our work in developing a tetraphenyl butadiene (TPB)-based detection system for a measurement of the neutron lifetime using magnetically confined ultracold neutrons (UCN). As part of the development of the detection system for this experiment, we studied the scintillation properties of liquid helium itself, characterized the fluorescent efficiencies of different fluors, and built and tested three detector geometries. We provide an overview of the results from these studies as well as references for additional information.

  16. Scintillation and luminescence in transparent colorless single and polycrystalline bulk ceramic ZnS

    SciTech Connect

    McCloy, John S.; Bliss, Mary; Miller, Brian W.; Wang, Zheming; Stave, Sean C.

    2015-01-01

    ZnS:Ag is a well-known extremely bright scintillator used in powder form for α-particle detection and, mixed with powdered LiF, for thermal neutron detection. Recently, we discovered some commercial bulk colorless and transparent, single-crystal and polycrystalline (chemical vapor-deposited) ZnS forms that scintillate in response to α-particles. The scintillation light transmits through the sample thickness (mm), challenging the commonly held assumption that ZnS is opaque to its own scintillation light. Individual α-particle events were imaged in space and time using a charged-particle camera originally developed for medical imaging applications. Photoluminescence (PL) and PL excitation show that scintillating bulk ZnS likely depends on different electronic defects than commercial ZnS powder scintillators. These defects, associated with copper and oxygen, are discussed in relation to PL results and extensive literature assessment. Commercial transparent ZnS is routinely produced by chemical vapor deposition to sizes larger than square meters, enabling potentially novel radiation detection applications requiring large, thick apertures.

  17. Development of novel growth methods for halide single crystals

    NASA Astrophysics Data System (ADS)

    Yokota, Yuui; Kurosawa, Shunsuke; Shoji, Yasuhiro; Ohashi, Yuji; Kamada, Kei; Yoshikawa, Akira

    2017-03-01

    We developed novel growth methods for halide scintillator single crystals with hygroscopic nature, Halide micro-pulling-down [H-μ-PD] method and Halide Vertical Bridgman [H-VB] method. The H-μ-PD method with a removable chamber system can grow a single crystal of halide scintillator material with hygroscopicity at faster growth rate than the conventional methods. On the other hand, the H-VB method can grow a large bulk single crystal of halide scintillator without a quartz ampule. CeCl3, LaBr3, Ce:LaBr3 and Eu:SrI2 fiber single crystals could be grown by the H-μ-PD method and Eu:SrI2 bulk single crystals of 1 and 1.5 inch in diameter could be grown by the H-VB method. The grown fiber and bulk single crystals showed comparable scintillation properties to the previous reports using the conventional methods.

  18. Gaseous photomultipliers for the readout of scintillators and detection Cherenkov radiation

    SciTech Connect

    Peskov, V.; Borovik-Romanov, A.

    1993-11-01

    The latest achievements in the development of gaseous detectors for registering UV and visible photons are described. Possible modifications of their design for some particular applications such as the readout of crystal scintillators. noble liquids, fibers and for large area Cherenkov detectors are discussed.

  19. Studies on Ca2+-Doped CeBr3 Scintillating Materials

    SciTech Connect

    Guss, P.; Foster, M. E.; Wong, B. M.; Doty, F. P.; Shah, K.; Squillante, M.; Glodo, J.; Yuan, D.

    2013-07-03

    Despite the outstanding scintillation performance characteristics of cerium tribromide (CeBr3) and cerium-activated lanthanum tribromide (LaBr3:Ce), their commercial availability and application is limited due to the difficulties of growing large, crack-free single crystals from these fragile materials. The objective of this investigation was to employ aliovalent doping to increase crystal strength while maintaining the optical properties of the crystal. One divalent dopant (Ca2+) was investigated as a dopant to strengthen CeBr3 without negatively impacting scintillation performance. Ingots containing nominal concentrations of 1.9% of the Ca2+ dopant were grown. Preliminary scintillation measurements are presented for this aliovalently doped scintillator. Ca2+-doped CeBr3 exhibited little or no change in the peak fluorescence emission for 371 nm optical excitation for CeBr3. The structural, electronic, and optical properties of CeBr3 crystals were investigated using the density functional theory within generalized gradient approximation. The calculated lattice parameters are in good agreement with the experimental data. The energy band structures and density of states were obtained. The optical properties of CeBr3, including the dielectric function, were calculated.

  20. Studies on Ca2+-Doped CeBr3 Scintillating Materials

    SciTech Connect

    Guss, P.; Foster, M. E.; Wong, B. M.; Doty, F. P.; Shah, K.; Squillante, M. R.; Shirwadkar, U.; Hawrami, R.; Tower, J.; Yuan, D.

    2013-09-01

    Despite the outstanding scintillation performance characteristics of cerium tribromide (CeBr3) and cerium-activated lanthanum tribromide (LaBr3:Ce), their commercial availability and application is limited due to the difficulties of growing large, crack-free single crystals from these fragile materials. The objective of this investigation was to employ aliovalent doping to increase crystal strength while maintaining the optical properties of the crystal. One divalent dopant (Ca2+) was investigated as a dopant to strengthen CeBr3 without negatively impacting scintillation performance. Ingots containing nominal concentrations of 1.9% of the Ca2+ dopant were grown. Preliminary scintillation measurements are presented for this aliovalently doped scintillator. Ca2+-doped CeBr3 exhibited little or no change in the peak fluorescence emission for 371 nm optical excitation for CeBr3. The structural, electronic, and optical properties of CeBr3 crystals were investigated using the density functional theory within generalized gradient approximation. The calculated lattice parameters are in good agreement with the experimental data. The energy band structures and density of states were obtained. The optical properties of CeBr3, including the dielectric function, were calculated.

  1. Low-energy neutron detector based upon lithium lanthanide borate scintillators

    DOEpatents

    Czirr, John B.

    1998-01-01

    An apparatus for detecting neutrons includes a cerium activated scintillation crystal containing .sup.10 B, with the scintillation crystal emitting light in response to .alpha. particles emitted from the .sup.10 B(n,.alpha.)Li* reaction. The apparatus also includes a gamma scintillator positioned adjacent the crystal and which generates light in response to gamma rays emitted from the decay of Li*. The apparatus further includes a first and a second light-to-electronic signal converter each positioned to respectively receive light from the crystal and the gamma scintillator, and each respectively outputting first and second electronic signals representative of .alpha. particles from the .sup.10 B(n,.alpha.)Li* reaction and gamma rays from the .sup.10 B(n,.alpha.)Li* reaction. The apparatus includes a coincidence circuit connected to receive the first and second signals and which generates a coincidence signal when the first and second signals coincide. The apparatus also includes a data analyzer for receiving an additional signal from at least one of the first and second converters, and for operating in response to the coincidence signal.

  2. Scintillation Forecasting Using NPOESS Data

    NASA Astrophysics Data System (ADS)

    Basu, B.; Retterer, J.; Demajistre, R.; de La Beaujardiere, O.; Scro, K.

    2005-12-01

    We have conducted a theoretical study of the use of NPOESS data for the forecasting of equatorial radio scintillation using knowledge of the equatorial Appleton anomaly, e.g., the peak-to-valley ratio of TEC (Total Electron Content) between the anomaly crests and the magnetic equator. The peak-to-valley ratio can be obtained from the UV (ultraviolet) imagery of the anomaly region that will be provided by the NPOESS sensors. The post-sunset enhancement of the upward drift velocity of the equatorial plasma has been shown, both theoretically and observationally, to be an important determinant of both the onset of scintillation and the strength of the anomaly. The technical approach is to run PBMOD, the AFRL low-latitude ionosphere model, with a range of post-sunset vertical drift velocities to determine the quantitative relationship between the peak-to-valley ratio and the maximum value of the pot-sunset upward drift velocity of equatorial plasma. Once the relationship is validated, it will be used to estimate the maximum value of the drift velocity from the peak-to-valley ratio, which is derived from the UV imagery data provided by NPOESS-like sensor, such as GUVI on TIMED satellite. The drift velocity will then be used in PBMOD to simulate the formation and evolution of equatorial plasma `bubbles' and calculate the distribution of the amplitude scintillation index S4. Results of the study will be discussed.

  3. A Review of Ionospheric Scintillation Models.

    PubMed

    Priyadarshi, S

    This is a general review of the existing climatological models of ionospheric radio scintillation for high and equatorial latitudes. Trans-ionospheric communication of radio waves from transmitter to user is affected by the ionosphere which is highly variable and dynamic in both time and space. Scintillation is the term given to irregular amplitude and phase fluctuations of the received signals and related to the electron density irregularities in the ionosphere. Key sources of ionospheric irregularities are plasma instabilities; every irregularities model is based on the theory of radio wave propagation in random media. It is important to understand scintillation phenomena and the approach of different theories. Therefore, we have briefly discussed the theories that are used to interpret ionospheric scintillation data. The global morphology of ionospheric scintillation is also discussed briefly. The most important (in our opinion) analytical and physical models of scintillation are reviewed here.

  4. Bridgman bulk growth and scintillation measurements of SrI2:Eu2+

    NASA Astrophysics Data System (ADS)

    Hawrami, R.; Glodo, J.; Shah, K. S.; Cherepy, N.; Payne, S.; Burger, A.; Boatner, L.

    2013-09-01

    Large diameter Bridgman growth of europium activated strontium iodide SrI2:Eu2+ produces crystals with light yield of up to 115,000 ph/MeV with an excellent light yield proportionality. SrI2:Eu2+ exhibits an outstanding energy resolution of better than 3% FWHM at 662 keV. Its emission is centered at 435 nm. The scintillation decays with a 1 μs time constant for small samples and up to 5 μs to larger crystals. This paper presents successful progress made in the vertical Bridgman crystal growth of SrI2:Eu2+ and its scintillator properties. Large diameter, crack-free and transparent SrI2:Eu2+single crystals with diameters of 1 in., 1.3 in., 1.5 in. and 2 in. were all successfully grown.

  5. Reflectivity quenching of ESR multilayer polymer film reflector in optically bonded scintillator arrays

    NASA Astrophysics Data System (ADS)

    Loignon-Houle, Francis; Pepin, Catherine M.; Charlebois, Serge A.; Lecomte, Roger

    2017-04-01

    The 3M-ESR multilayer polymer film is a widely used reflector in scintillation detector arrays. As specified in the datasheet and confirmed experimentally by measurements in air, it is highly reflective (> 98 %) over the entire visible spectrum (400-1000 nm) for all angles of incidence. Despite these outstanding characteristics, it was previously found that light crosstalk between pixels in a bonded LYSO scintillator array with ESR reflector can be as high as ∼30-35%. This unexplained light crosstalk motivated further investigation of ESR optical performance. Analytical simulation of a multilayer structure emulating the ESR reflector showed that the film becomes highly transparent to incident light at large angles when surrounded on both sides by materials of refractive index higher than air. Monte Carlo simulations indicate that a considerable fraction (∼25-35%) of scintillation photons are incident at these leaking angles in high aspect ratio LYSO scintillation crystals. The film transparency was investigated experimentally by measuring the scintillation light transmission through the ESR film sandwiched between a scintillation crystal and a photodetector with or without layers of silicone grease. Strong light leakage, up to nearly 30%, was measured through the reflector when coated on both sides with silicone, thus elucidating the major cause of light crosstalk in bonded arrays. The reflector transparency was confirmed experimentally for angles of incidence larger than 60 ° using a custom designed setup allowing illumination of the bonded ESR film at selected grazing angles. The unsuspected ESR film transparency can be beneficial for detector arrays exploiting light sharing schemes, but it is highly detrimental for scintillator arrays designed for individual pixel readout.

  6. Neutron response characterization for an EJ299-33 plastic scintillation detector

    SciTech Connect

    Lawrence, Chris C.; Febbraro, Michael; Massey, Thomas N.; Flaska, Marek; Becchetti, F. D.; Pozzi, Sara A.

    2014-05-10

    Organic scintillation detectors have shown promise as neutron detectors for characterizing special nuclear materials in various arms-control and homeland security applications. Recent advances have yielded a new plastic scintillator - EJ299-33 - with pulse-shape-discrimination (PSD) capability. Plastic scintillators would have a much expanded range of deployment relative to liquids and crystals. Here, we present a full characterization of pulse height response to fission-energy neutrons for an EJ299-33 detector with 7.62-by-7.62-cm cylindrical active volume, and compare with an EJ309 liquid scintillator in the same assembly. Scintillation light output relations, energy resolutions, and response matrices are presented for both detectors. A Continuous spectrum neutron source, obtained via the bombardment of Al-27 with 7.44-MeV deuterons at the Edwards Accelerator Facility at Ohio University, was used for the measurement. A new procedure for evaluating and comparing PSD performance is presented which accounts for the effect of the light output relation on the ability to detect low energy neutrons. The EJ299-33 is shown to have considerable deficit in matrix condition, and in PSD figure of merit when compared to EJ309, especially when neutron energy is taken into account. Furthermore the EJ299 is likely to bring a modest PSD capability into a array of held applications that are not accessible to liquids or crystals. (C) 2014 Elsevier B.V. All rights reserved. Keywords

  7. Neutron response characterization for an EJ299-33 plastic scintillation detector

    DOE PAGES

    Lawrence, Chris C.; Febbraro, Michael; Massey, Thomas N.; ...

    2014-05-10

    Organic scintillation detectors have shown promise as neutron detectors for characterizing special nuclear materials in various arms-control and homeland security applications. Recent advances have yielded a new plastic scintillator - EJ299-33 - with pulse-shape-discrimination (PSD) capability. Plastic scintillators would have a much expanded range of deployment relative to liquids and crystals. Here, we present a full characterization of pulse height response to fission-energy neutrons for an EJ299-33 detector with 7.62-by-7.62-cm cylindrical active volume, and compare with an EJ309 liquid scintillator in the same assembly. Scintillation light output relations, energy resolutions, and response matrices are presented for both detectors. A Continuousmore » spectrum neutron source, obtained via the bombardment of Al-27 with 7.44-MeV deuterons at the Edwards Accelerator Facility at Ohio University, was used for the measurement. A new procedure for evaluating and comparing PSD performance is presented which accounts for the effect of the light output relation on the ability to detect low energy neutrons. The EJ299-33 is shown to have considerable deficit in matrix condition, and in PSD figure of merit when compared to EJ309, especially when neutron energy is taken into account. Furthermore the EJ299 is likely to bring a modest PSD capability into a array of held applications that are not accessible to liquids or crystals. (C) 2014 Elsevier B.V. All rights reserved. Keywords« less

  8. Recording of relativistic particles in thin scintillators

    SciTech Connect

    Tolstukhin, I A.; Somov, Alexander S.; Somov, S. V.; Bolozdynya, A. I.

    2014-11-01

    Results of investigating an assembly of thin scintillators and silicon photomultipliers for registering relativistic particles with the minimum ionization are presented. A high efficiency of registering relativistic particles using an Ej-212 plastic scintillator, BSF-91A wavelength-shifting fiber (Saint-Gobain), and a silicon photomultiplier (Hamamtsu) is shown. The measurement results are used for creating a scintillation hodoscope of the magnetic spectrometer for registering γ quanta in the GlueX experiment.

  9. Scintillator tiles read out with silicon photomultipliers

    NASA Astrophysics Data System (ADS)

    Pooth, O.; Radermacher, T.; Weingarten, S.; Weinstock, L.

    2015-10-01

    A detector prototype based on a fast plastic scintillator read out with silicon photomultipliers is presented. All studies have been done with cosmic muons and focus on parameter optimization such as coupling the SiPM to the scintillator or wrapping the scintillator with reflective material. The prototype shows excellent results regarding the light-yield and offers a detection efficiency of 99.5% with a signal purity of 99.9% for cosmic muons.

  10. Spacecraft Radio Scintillation and Solar System Exploration

    NASA Technical Reports Server (NTRS)

    Woo, Richard

    1993-01-01

    When a wave propagates through a turbulent medium, scattering by the random refractive index inhomogeneities can lead to a wide variety of phenomena that have been the subject of extensive study. The observed scattering effects include amplitude or intensity scintillation, phase scintillation, angular broadening, and spectral broadening, among others. In this paper, I will refer to these scattering effects collectively as scintillation. Although the most familiar example is probably the twinkling of stars (light wave intensity scintillation by turbulence in the Earth's atmosphere), scintillation has been encountered and investigated in such diverse fields as ionospheric physics, oceanography, radio astronomy, and radio and optical communications. Ever since planetary spacecraft began exploring the solar system, scintillation has appeared during the propagation of spacecraft radio signals through planetary atmospheres, planetary ionospheres, and the solar wind. Early studies of these phenomena were motivated by the potential adverse effects on communications and navigation, and on experiments that use the radio link to conduct scientific investigations. Examples of the latter are radio occultation measurements (described below) of planetary atmospheres to deduce temperature profiles, and the search for gravitational waves. However,these concerns soon gave way to the emergence of spacecraft radio scintillation as a new scientific tool for exploring small-scale dynamics in planetary atmospheres and structure in the solar wind, complementing in situ and other remote sensing spacecraft measurements, as well as scintillation measurements using natural (celestial) radio sources. The purpose of this paper is to briefly describe and review the solar system spacecraft radio scintillation observations, to summarize the salient features of wave propagation analyses employed in interpreting them, to underscore the unique remote sensing capabilities and scientific relevance of

  11. Scintillation properties of pure CaF 2

    NASA Astrophysics Data System (ADS)

    Mikhailik, V. B.; Kraus, H.; Imber, J.; Wahl, D.

    2006-10-01

    The temperature dependence of the decay time and scintillation light yield of pure CaF 2 crystal was measured over the temperature range 8-305 K using the multiphoton coincidence counting technique. Pure CaF 2 exhibits emission of triplet self-trapped excitons at 280 nm with a slow decay, the time constant of which changes significantly with temperature. The main decay time constant increases by three orders of magnitude when cooled, from 0.96±0.06 μs at 295 K to 930±40 μs at 8 K. The results obtained demonstrate that the scintillation light yield of pure CaF 2 increases with decreasing temperature down to 20 K below which it is roughly constant. At low temperatures the light yield of CaF 2 is estimated to be 60% relative to that of pure CaWO 4. It is concluded that undoped calcium fluoride is a very attractive target material for experimental searches for rare events based on the detection of phonon and scintillation signals.

  12. Waveshifters and Scintillators for Ionizing Radiation Detection

    SciTech Connect

    B.Baumgaugh; J.Bishop; D.Karmgard; J.Marchant; M.McKenna; R.Ruchti; M.Vigneault; L.Hernandez; C.Hurlbut

    2007-12-11

    Scintillation and waveshifter materials have been developed for the detection of ionizing radiation in an STTR program between Ludlum Measurements, Inc. and the University of Notre Dame. Several new waveshifter materials have been developed which are comparable in efficiency and faster in fluorescence decay than the standard material Y11 (K27) used in particle physics for several decades. Additionally, new scintillation materials useful for fiber tracking have been developed which have been compared to 3HF. Lastly, work was done on developing liquid scintillators and paint-on scintillators and waveshifters for high radiation environments.

  13. Radio wave scintillations at equatorial regions

    NASA Technical Reports Server (NTRS)

    Poularikas, A. D.

    1972-01-01

    Radio waves, passing through the atmosphere, experience amplitude and phase fluctuations know as scintillations. A characterization of equatorial scintillation, which has resulted from studies of data recorded primarily in South America and equatorial Africa, is presented. Equatorial scintillation phenomena are complex because they appear to vary with time of day (pre-and postmidnight), season (equinoxes), and magnetic activity. A wider and more systematic geographical coverage is needed for both scientific and engineering purposes; therefore, it is recommended that more observations should be made at earth stations (at low-geomagnetic latitudes) to record equatorial scintillation phenomena.

  14. A multi-channel setup to study fractures in scintillators

    NASA Astrophysics Data System (ADS)

    Tantot, A.; Bouard, C.; Briche, R.; Lefèvre, G.; Manier, B.; Zaïm, N.; Deschanel, S.; Vanel, L.; Di Stefano, P. C. F.

    2016-12-01

    To investigate fractoluminescence in scintillating crystals used for particle detection, we have developed a multi-channel setup built around samples of double-cleavage drilled compression (DCDC) geometry in a controllable atmosphere. The setup allows the continuous digitization over hours of various parameters, including the applied load, and the compressive strain of the sample, as well as the acoustic emission. Emitted visible light is recorded with nanosecond resolution, and crack propagation is monitored using infrared lighting and camera. An example of application to \\text{B}{{\\text{i}}4}\\text{G}{{\\text{e}}3}{{\\text{O}}12} (BGO) is provided.

  15. PREFACE: Applications of Novel Scintillators for Research and Industry (ANSRI 2015)

    NASA Astrophysics Data System (ADS)

    Roberts, O. J.

    2015-06-01

    Scintillator detectors are used widely in the field of γ- and X-ray spectroscopy, particularly in the mid 1900s when the invention of NaI(Tl) by nobel laureate Robert Hofstadter in 1948, spurred the creation of new scintillator materials. In the development of such new scintillators, important characteristics such as its intrinsic efficiency, position sensitivity, robustness, energy and timing response, light output, etc, need to be addressed. To date, these requirements cannot be met by a single type of scintillator alone and therefore the development of an ''ideal'' scintillator remains the holy grail of nuclear instrumentation. Consequently, the last two decades have seen significant progress in the development of scintillator crystals, driven largely by technological advances. Conventional inorganic scintillators such as NaI(Tl) and BGO are now being replaced with better, novel organic, inorganic, ceramic and plastic scintillators offering a wider variety of options for many applications. The workshop on the Applications of Novel Scintillators in Research and Industry was held at University College Dublin in January 2015 and covered a wide range of topics that characterise modern advances in the field of scintillator technology. This set of proceedings covers areas including the growth, production and characterisation of such contemporary scintillators, along with their applications in various fields, such as; Medical Imaging; Defence/Security; Astrophysics; and Nuclear/Particle Physics. We would like to thank all those who presented their recent results on their research at the workshop. These proceedings atest to the excitement and interest in such a broad field, that pervades the pursuit of the development of novel materials for future applications. We would also like to thank Professor Luigi Piro, for giving an interesting public talk during the conference, and to the Institute of Physics Ireland Group for supporting the event. We thank ORTEC for

  16. Ruby-based inorganic scintillation detectors for 192Ir brachytherapy

    NASA Astrophysics Data System (ADS)

    Kertzscher, Gustavo; Beddar, Sam

    2016-11-01

    We tested the potential of ruby inorganic scintillation detectors (ISDs) for use in brachytherapy and investigated various unwanted luminescence properties that may compromise their accuracy. The ISDs were composed of a ruby crystal coupled to a poly(methyl methacrylate) fiber-optic cable and a charge-coupled device camera. The ISD also included a long-pass filter that was sandwiched between the ruby crystal and the fiber-optic cable. The long-pass filter prevented the Cerenkov and fluorescence background light (stem signal) induced in the fiber-optic cable from striking the ruby crystal, which generates unwanted photoluminescence rather than the desired radioluminescence. The relative contributions of the radioluminescence signal and the stem signal were quantified by exposing the ruby detectors to a high-dose-rate brachytherapy source. The photoluminescence signal was quantified by irradiating the fiber-optic cable with the detector volume shielded. Other experiments addressed time-dependent luminescence properties and compared the ISDs to commonly used organic scintillator detectors (BCF-12, BCF-60). When the brachytherapy source dwelled 0.5 cm away from the fiber-optic cable, the unwanted photoluminescence was reduced from  >5% to  <1% of the total signal as long as the ISD incorporated the long-pass filter. The stem signal was suppressed with a band-pass filter and was  <3% as long as the source distance from the scintillator was  <7 cm. Some ruby crystals exhibited time-dependent luminescence properties that altered the ruby signal by  >5% within 10 s from the onset of irradiation and after the source had retracted. The ruby-based ISDs generated signals of up to 20 times that of BCF-12-based detectors. The study presents solutions to unwanted luminescence properties of ruby-based ISDs for high-dose-rate brachytherapy. An optic filter should be sandwiched between the ruby crystal and the fiber-optic cable to suppress the

  17. Comparison of the imaging performances for recently developed monolithic scintillators: CRY018 and CRY019 for dual isotope gamma ray imaging applications

    NASA Astrophysics Data System (ADS)

    Polito, C.; Pani, R.; Trigila, C.; Cinti, M. N.; Fabbri, A.; Frantellizzi, V.; De Vincentis, G.; Pellegrini, R.; Pani, R.

    2017-01-01

    The growing interest for new scintillation crystals with outstanding imaging performances (i.e. resolution and efficiency) has suggested the study of recently discovered scintillators named CRY018 and CRY019. The crystals under investigation are monolithic and have shown enhanced characteristics both for gamma ray spectrometry and for Nuclear Medicine imaging applications such as the dual isotope imaging. Moreover, the non-hygroscopic nature and the absence of afterglow make these scintillators even more attractive for the potential improvement in a wide range of applications. These scintillation crystals show a high energy resolution in the energy range involved in Nuclear Medicine, allowing the discrimination between very close energy values. Moreover, in order to prove their suitability of being powerful imaging systems, the imaging performances like the position linearity and the intrinsic spatial resolution have been evaluated obtaining satisfactory results thanks to the implementation of an optimized algorithm for the images reconstruction.

  18. Scintillation properties of Pr-activated LuAlO 3

    NASA Astrophysics Data System (ADS)

    Drozdowski, Winicjusz; Wojtowicz, Andrzej J.; Wiśniewski, Dariusz; Łukasiewicz, Tadeusz; Kisielewski, Jarosław

    2006-01-01

    Praseodymium activated LuAlO 3 (LuAP) crystals have been grown using the Czochralski method at ITME, Warsaw. In this communication the measurements of radioluminescence (RL), low temperature thermoluminescence (TL), room temperature afterglow (AG), scintillation light yields (LY), and scintillation time profiles (STP), performed on polished 2 × 2 × 10 mm pixels with three Pr concentrations (0.003, 0.04, and 0.08 at.%), are reported. Two sets of samples are compared: (i) "as grown", and (ii) annealed in H 2 atmosphere.

  19. X-ray luminescence based spectrometer for investigation of scintillation properties

    SciTech Connect

    Varney, C. R.; Khamehchi, M. A.; Ji, Jianfeng; Selim, F. A.

    2012-10-15

    A new x-ray luminescence based spectrometer was developed and installed to examine the scintillation properties of materials while revealing the origins of luminescence and investigating trapping defects. Measurements were performed on a number of undoped and Ce doped yttrium aluminum garnet crystals and various luminescence centers were characterized. The measured x-ray luminescence spectra provide information about the spectral range and the scintillation efficiency and linearity. The efficiency of charge-carriers production due to x ray, their energy transfer to the luminescence centers, and the efficiency of luminescence are all reflected in the efficiency of x-ray luminescence.

  20. Testing a new NIF neutron time-of-flight detector with a bibenzyl scintillator on OMEGA.

    PubMed

    Glebov, V Yu; Forrest, C; Knauer, J P; Pruyne, A; Romanofsky, M; Sangster, T C; Shoup, M J; Stoeckl, C; Caggiano, J A; Carman, M L; Clancy, T J; Hatarik, R; McNaney, J; Zaitseva, N P

    2012-10-01

    A new neutron time-of-flight (nTOF) detector with a bibenzyl crystal as a scintillator has been designed and manufactured for the National Ignition Facility (NIF). This detector will replace a nTOF20-Spec detector with an oxygenated xylene scintillator currently operational on the NIF to improve the areal-density measurements. In addition to areal density, the bibenzyl detector will measure the D-D and D-T neutron yield and the ion temperature of indirect- and direct-drive-implosion experiments. The design of the bibenzyl detector and results of tests on the OMEGA Laser System are presented.

  1. Photodetectors for Scintillator Proportionality Measurement

    SciTech Connect

    Moses, William W.; Choong, Woon-Seng; Hull, Giulia; Payne, Steve; Cherepy, Nerine; Valentine, J.D.

    2010-10-18

    We evaluate photodetectors for use in a Compton Coincidence apparatus designed for measuring scintillator proportionality. There are many requirements placed on the photodetector in these systems, including active area, linearity, and the ability to accurately measure low light levels (which implies high quantum efficiency and high signal-to-noise ratio). Through a combination of measurement and Monte Carlo simulation, we evaluate a number of potential photodetectors, especially photomultiplier tubes and hybrid photodetectors. Of these, we find that the most promising devices available are photomultiplier tubes with high ({approx}50%) quantum efficiency, although hybrid photodetectors with high quantum efficiency would be preferable.

  2. Current status on plastic scintillators modifications

    SciTech Connect

    Hamel, Matthieu; Bertrand, Guillaume H.V.; Carrel, Frederick; Coulon, Romain; Dumazert, Jonathan; Montbarbon, Eva; Sguerra, Fabien

    2015-07-01

    Recent developments of plastic scintillators are reviewed, from 2000 to March 2015. All examples are distributed into the main purpose, i.e. the nature of the radionuclide provided with the scope of detection of various radiation particles. The main characteristics of these newly created scintillators and their detection properties are given. (authors)

  3. Binderless composite scintillator for neutron detection

    DOEpatents

    Hodges, Jason P [Knoxville, TN; Crow, Jr; Lowell, M [Oak Ridge, TN; Cooper, Ronald G [Oak Ridge, TN

    2009-03-10

    Composite scintillator material consisting of a binderless sintered mixture of a Lithium (Li) compound containing .sup.6Li as the neutron converter and Y.sub.2SiO.sub.5:Ce as the scintillation phosphor, and the use of this material as a method for neutron detection. Other embodiments of the invention include various other Li compounds.

  4. Epoxy resins produce improved plastic scintillators

    NASA Technical Reports Server (NTRS)

    Markley, F. W.

    1967-01-01

    Plastic scintillator produced by the substitution of epoxy resins for the commonly used polystyrene is easy to cast, stable at room temperature, and has the desirable properties of a thermoset or cross-linked system. Such scintillators can be immersed directly in strong solvents, an advantage in many chemical and biological experiments.

  5. Scintillator handbook with emphasis on cesium iodide

    NASA Technical Reports Server (NTRS)

    Tidd, J. L.; Dabbs, J. R.; Levine, N.

    1973-01-01

    This report provides a background of reasonable depth and reference material on scintillators in general. Particular attention is paid to the cesium iodide scintillators as used in the High Energy Astronomy Observatory (HEAO) experiments. It is intended especially for use by persons such as laboratory test personnel who need to obtain a working knowledge of these materials and their characteristics in a short time.

  6. Atmospheric Neutron Measurements using a Small Scintillator Based Detector

    NASA Astrophysics Data System (ADS)

    Kole, Merlin; Pearce, Mark; Fukazawa, Yasushi; Fukuda, Kentaro; Ishizu, Sumito; Jackson, Miranda; Kamae, Tune; Kawaguchi, Noriaki; Kawano, Takafumi; Kiss, Mozsi; Moretti, Elena; Yanagida, Takayuki; Chauvin, Maxime; Mikhalev, Victor; Rydstrom, Stefan; Takahashi, Hiromitsu

    PoGOLino is a standalone scintillator-based neutron detector designed for balloon-borne missions. Its main purpose is to provide data of the neutron flux in 2 different energy ranges in the high altitude / high latitude region where the highest neutron flux in the atmosphere is found. Furthermore the influence of the Solar activity upon the neutron environment in this region is relatively strong. As a result both short and long term time fluctuations are strongest in this region. At high altitudes neutrons can form a source of background for balloon-borne scientific measurements. They can furthermore form a major source for single event upsets in electronics. A good understanding of the high altitude / high latitude neutron environment is therefore important. Measurements of the neutron environment in this region are however lacking. PoGOLino contains two 5 mm thick Lithium Calcium Aluminium Fluoride (LiCAF) scintillators used for neutron detection. The LiCAF crystals are sandwiched between 2 Bismuth Germanium Oxide (BGO) scintillating crystals, which serve to veto signals produced by gamma-rays and charged particles. The veto system makes measurements of the neutron flux possible even in high radiation environments. One LiCAF detector is shielded with polyethylene while the second remains unshielded, making the detectors sensitive in different energy ranges. The choice of a scintillator crystals as the detection material ensures a high detection efficiency while keeping the instrument small, robust and light weight. The full standalone cylindrical instrument has a radius of 120 mm, a height of 670 mm and a total mass of 13 kg, making it suitable as a piggy back mission. PoGOLino was successfully launched on March 20th 2013 from the Esrange Space Center in Northern Sweden to an altitude of 30.9 km. A detailed description of the detector design is presented, along with results of of the flight. The neutron flux measured during flight is compared to predictions based

  7. Extruded scintillator for the calorimetry applications

    SciTech Connect

    Dyshkant, A.; Rykalin, V.; Pla-Dalmau, A.; Beznosko, D.; /SUNY, Stony Brook

    2006-08-01

    An extrusion line has been installed and successfully operated at FNAL (Fermi National Accelerator Laboratory) in collaboration with NICADD (Northern Illinois Center for Accelerator and Detector Development). This new Facility will serve to further develop and improve extruded plastic scintillator. Recently progress has been made in producing co-extruded plastic scintillator, thus increasing the potential HEP applications of this Facility. The current R&D work with extruded and co-extruded plastic scintillator for a potential ALICE upgrade, the ILC calorimetry program and the MINERvA experiment show the attractiveness of the chosen strategy for future experiments and calorimetry. We extensively discuss extruded and co-extruded plastic scintillator in calorimetry in synergy with new Solid State Photomultipliers. The characteristics of extruded and co-extruded plastic scintillator will be presented here as well as results with non-traditional photo read-out.

  8. Extruded scintillator for the Calorimetry applications

    NASA Astrophysics Data System (ADS)

    Dyshkant, A.; Rykalin, V.; Pla-Dalmau, A.; Beznosko, D.

    2006-10-01

    An extrusion line has been installed and successfully operated at FNAL (Fermi National Accelerator Laboratory) in collaboration with NICADD (Northern Illinois Center for Accelerator and Detector Development). This new Facility will serve to further develop and improve extruded plastic scintillator. Recently progress has been made in producing co-extruded plastic scintillator, thus increasing the potential HEP applications of this Facility. The current R&D work with extruded and co-extruded plastic scintillator for a potential ALICE upgrade, the ILC calorimetry program and the MINERvA experiment show the attractiveness of the chosen strategy for future experiments and calorimetry. We extensively discuss extruded and co-extruded plastic scintillator in calorimetry in synergy with new Solid State Photomultipliers. The characteristics of extruded and co-extruded plastic scintillator will be presented here as well as results with non-traditional photo read-out.

  9. Scintillation Effects on Space Shuttle GPS Data

    NASA Technical Reports Server (NTRS)

    Goodman, John L.; Kramer, Leonard

    2001-01-01

    Irregularities in ionospheric electron density result in variation in amplitude and phase of Global Positioning System (GPS) signals, or scintillation. GPS receivers tracking scintillated signals may lose carrier phase or frequency lock in the case of phase sc intillation. Amplitude scintillation can cause "enhancement" or "fading" of GPS signals and result in loss of lock. Scintillation can occur over the equatorial and polar regions and is a function of location, time of day, season, and solar and geomagnetic activity. Mid latitude regions are affected only very rarely, resulting from highly disturbed auroral events. In the spring of 1998, due to increasing concern about scintillation of GPS signals during the upcoming solar maximum, the Space Shuttle Program began to assess the impact of scintillation on Collins Miniaturized Airborne GPS Receiver (MAGR) units that are to replace Tactical Air Control and Navigation (TACAN) units on the Space Shuttle orbiters. The Shuttle Program must determine if scintillation effects pose a threat to safety of flight and mission success or require procedural and flight rule changes. Flight controllers in Mission Control must understand scintillation effects on GPS to properly diagnose "off nominal" GPS receiver performance. GPS data from recent Space Shuttle missions indicate that the signals tracked by the Shuttle MAGR manifest scintillation. Scintillation is observed as anomalous noise in velocity measurements lasting for up to 20 minutes on Shuttle orbit passes and are not accounted for in the error budget of the MAGR accuracy parameters. These events are typically coincident with latitude and local time occurrence of previously identified equatorial spread F within about 20 degrees of the magnetic equator. The geographic and seasonal history of these events from ground-based observations and a simple theoretical model, which have potential for predicting events for operational purposes, are reviewed.

  10. Temperature dependence of CsI(Tl) gamma-ray excited scintillation characteristics

    SciTech Connect

    Not Available

    1993-10-01

    Gamma-ray excited emission spectrum, absolute scintillation yield, rise and decay time constants, and thermoluminescence emissions of CsI(Tl) were measured at {minus}100 to +50 C, for crystals from 4 different vendors. The thermoluminescence glow curves were the only property that varied significantly from crystal to crystal; room temperature operation in current mode could be susceptible to temperature fluctuations. The CsI(Tl) emission spectrum has emission bands peaking around 400 and 560 nm; the former band disappears between {minus}50 and {minus}75 C. The RT absolute scintillation yield was calculated to be 65,500{plus_minus}4,100 photons/MeV. The two primary decay time constants increases about exponentially with inverse temperature. An ultra-fast decay component was confirmed. Applications are discussed.

  11. Simulation of optical interstellar scintillation

    NASA Astrophysics Data System (ADS)

    Habibi, F.; Moniez, M.; Ansari, R.; Rahvar, S.

    2013-04-01

    Aims: Stars twinkle because their light propagates through the atmosphere. The same phenomenon is expected on a longer time scale when the light of remote stars crosses an interstellar turbulent molecular cloud, but it has never been observed at optical wavelengths. The aim of the study described in this paper is to fully simulate the scintillation process, starting from the molecular cloud description as a fractal object, ending with the simulations of fluctuating stellar light curves. Methods: Fast Fourier transforms are first used to simulate fractal clouds. Then, the illumination pattern resulting from the crossing of background star light through these refractive clouds is calculated from a Fresnel integral that also uses fast Fourier transform techniques. Regularisation procedure and computing limitations are discussed, along with the effect of spatial and temporal coherency (source size and wavelength passband). Results: We quantify the expected modulation index of stellar light curves as a function of the turbulence strength - characterised by the diffraction radius Rdiff - and the projected source size, introduce the timing aspects, and establish connections between the light curve observables and the refractive cloud. We extend our discussion to clouds with different structure functions from Kolmogorov-type turbulence. Conclusions: Our study confirms that current telescopes of ~4 m with fast-readout, wide-field detectors have the capability of discovering the first interstellar optical scintillation effects. We also show that this effect should be unambiguously distinguished from any other type of variability through the observation of desynchronised light curves, simultaneously measured by two distant telescopes.

  12. The COSINUS project: perspectives of a NaI scintillating calorimeter for dark matter search

    NASA Astrophysics Data System (ADS)

    Angloher, G.; Carniti, P.; Cassina, L.; Gironi, L.; Gotti, C.; Gütlein, A.; Hauff, D.; Maino, M.; Nagorny, S. S.; Pagnanini, L.; Pessina, G.; Petricca, F.; Pirro, S.; Pröbst, F.; Reindl, F.; Schäffner, K.; Schieck, J.; Seidel, W.

    2016-08-01

    The R&D project COSINUS (Cryogenic Observatory for SIgnatures seen in Next-generation Underground Searches) aims to develop a cryogenic scintillating calorimeter using an undoped NaI-crystal as target for direct dark matter search. Dark matter particles interacting with the detector material generate both a phonon signal and scintillation light. While the phonon signal provides a precise determination of the deposited energy, the simultaneously measured scintillation light allows for particle identification on an event-by-event basis, a powerful tool to study material-dependent interactions, and to suppress backgrounds. Using the same target material as the DAMA/LIBRA collaboration, the COSINUS technique may offer a unique possibility to investigate and contribute information to the presently controversial situation in the dark matter sector. We report on the dedicated design planned for the NaI proof-of-principle detector and the objectives of using this detection technique in the light of direct dark matter detection.

  13. Quantitative low-energy ion beam characterization by beam profiling and imaging via scintillation screens

    NASA Astrophysics Data System (ADS)

    Germer, S.; Pietag, F.; Polak, J.; Arnold, T.

    2016-11-01

    This study presents the imaging and characterization of low-current ion beams in the neutralized state monitored via single crystal YAG:Ce (Y3Al5O12) scintillators. To validate the presented beam diagnostic tool, Faraday cup measurements and test etchings were performed. Argon ions with a typical energy of 1.0 keV were emitted from an inductively coupled radio-frequency (13.56 MHz) ion beam source with total currents of some mA. Different beam properties, such as, lateral ion current density, beam divergence angle, and current density in pulsed ion beams have been studied to obtain information about the spatial beam profile and the material removal rate distribution. We observed excellent imaging properties with the scintillation screen and achieved a detailed characterization of the neutralized ion beam. A strong correlation between the scintillator light output, the ion current density, and the material removal rate could be observed.

  14. Considerations on thermal effects in doped scintillators for dark matter and other rare events searches

    NASA Astrophysics Data System (ADS)

    Chapellier, M.

    2009-08-01

    The scintillation properties of luminescent crystals are well known at room temperature. It is only recently, for the sake of dark matter and rare events searches that the studies have been extended to very low temperatures in the millikelvin range. Some little-known facts on the behaviour of bolometers , and more specifically on scintillating ones, are recalled in a simple manner. A few experiments to better understand them are proposed. The term bolometer is used here for calorimeter. Normally a bolometer will measure a flux of energy whereas a calorimeter measures a deposited energy. The tendency is to use bolometer for both types of measurement. A germanium bolometer does not measure the total energy received, part of it is transformed in ionization energy. The same is true for scintillating bolometer.

  15. High-light-output scintillator for photodiode readout: LuI3:Ce3+

    NASA Astrophysics Data System (ADS)

    Birowosuto, M. D.; Dorenbos, P.; van Eijk, C. W. E.; Krämer, K. W.; Güdel, H. U.

    2006-06-01

    In this paper, we investigated the scintillation properties of LuI3:Ce3+. Radioluminescence, light output, energy resolution, and γ-scintillation decay are reported. We find an extremely high light output of 98 000+/-10 000 photons/MeV. LuI3:Ce3+ also gives a very high electron-hole (e-h) pair response when it is coupled with an avalanche photodiode (APD) (92 000+/-9000 e-h pairs/MeV). With an APD, a best energy resolution (full width at half maximum over the peak position) of 3.3%+/-0.3% for 662 keV γ quanta is observed. A combination of an extremely high light output and a good energy resolution makes LuI3:Ce3+ an ideal scintillator for radiation sensor applications. Some drawbacks due to the hygroscopicity and the difficult growth of LuI3:Ce3+ crystals are also discussed.

  16. Performance characterization of a new high resolution PET scintillation detector

    PubMed Central

    Foudray, A M K; Olcott, P D

    2013-01-01

    Performance of a new high resolution PET detection concept is presented. In this new concept, annihilation radiation enters the scintillator detectors edge-on. Each detector module comprises two 8 × 8 LYSO scintillator arrays of 0.91 × 0.91 × 1 mm3 crystals coupled to two position-sensitive avalanche photodiodes (PSAPDs) mounted on a flex circuit. Appropriate crystal segmentation allows the recording of all three spatial coordinates of the interaction(s) simultaneously with submillimeter resolution. We report an average energy resolution of 14.6 ± 1.7% for 511 keV photons at FWHM. Coincident time resolution was determined to be 2.98 ± 0.13 ns FWHM on average. The coincidence point spread function (PSF) has an average FWHM of 0.837 ± 0.049 mm (using a 500 μm spherical source) and is uniform across the arrays. Both PSF and coincident time resolution degrade when Compton interactions are included in the data. Different blurring factors were evaluated theoretically, resulting in a calculated PSF of 0.793 mm, in good agreement with the measured value. PMID:20844332

  17. Femtosecond laser ablation of cadmium tungstate for scintillator arrays

    NASA Astrophysics Data System (ADS)

    Richards, S.; Baker, M. A.; Wilson, M. D.; Lohstroh, A.; Seller, P.

    2016-08-01

    Ultrafast pulsed laser ablation has been investigated as a technique to machine CdWO4 single crystal scintillator and segment it into small blocks with the aim of fabricating a 2D high energy X-ray imaging array. Cadmium tungstate (CdWO4) is a brittle transparent scintillator used for the detection of high energy X-rays and γ-rays. A 6 W Yb:KGW Pharos-SP pulsed laser of wavelength 1028 nm was used with a tuneable pulse duration of 10 ps to 190 fs, repetition rate of up to 600 kHz and pulse energies of up to 1 mJ was employed. The effect of varying the pulse duration, pulse energy, pulse overlap and scan pattern on the laser induced damage to the crystals was investigated. A pulse duration of ≥500 fs was found to induce substantial cracking in the material. The laser induced damage was minimised using the following operating parameters: a pulse duration of 190 fs, fluence of 15.3 J cm-2 and employing a serpentine scan pattern with a normalised pulse overlap of 0.8. The surface of the ablated surfaces was studied using scanning electron microscopy, energy dispersive X-ray spectroscopy, atomic force microscopy and X-ray photoelectron spectroscopy. Ablation products were found to contain cadmium tungstate together with different cadmium and tungsten oxides. These laser ablation products could be removed using an ammonium hydroxide treatment.

  18. Cesium hafnium chloride scintillator coupled with an avalanche photodiode photodetector

    NASA Astrophysics Data System (ADS)

    Kurosawa, S.; Kodama, S.; Yokota, Y.; Horiai, T.; Yamaji, A.; Shoji, Y.; Král, R.; Pejchal, J.; Ohashi, Y.; Kamada, K.; Nikl, M.; Yoshikawa, A.

    2017-02-01

    Optical and scintillation properties of pure Cs2HfCl6 (CHC) single crystals were investigated. In particular, light output and energy resolution were measured using a Si avalanche photodiode (Si-APD), since the Si-APD has sufficient quantum efficiency of around 70 % at emission wavelength region of CHC around 420 nm. This CHC single crystal grown using the vertical Bridgeman method showed light output of 37,000± 2,000 photons/MeV . The FWHM energy resolution was determined to be 3.7± 0.5× (E/662 keV)‑0.85± 0.03[%], where E [keV] is the gamma-ray energy. Moreover, the temperature dependence of the light output was stable from ‑5 to 30 oC, while the light output increased below ‑10 oC.

  19. Measurement of radiation damage of water-based liquid scintillator and liquid scintillator

    DOE PAGES

    Bignell, L. J.; Diwan, M. V.; Hans, S.; ...

    2015-10-19

    Liquid scintillating phantoms have been proposed as a means to perform real-time 3D dosimetry for proton therapy treatment plan verification. We have studied what effect radiation damage to the scintillator will have upon this application. We have performed measurements of the degradation of the light yield and optical attenuation length of liquid scintillator and water-based liquid scintillator after irradiation by 201 MeV proton beams that deposited doses of approximately 52 Gy, 300 Gy, and 800 Gy in the scintillator. Liquid scintillator and water-based liquid scintillator (composed of 5% scintillating phase) exhibit light yield reductions of 1.74 ± 0.55 % andmore » 1.31 ± 0.59 % after ≈ 800 Gy of proton dose, respectively. Some increased optical attenuation was observed in the irradiated samples, the measured reduction to the light yield is also due to damage to the scintillation light production. Based on our results and conservative estimates of the expected dose in a clinical context, a scintillating phantom used for proton therapy treatment plan verification would exhibit a systematic light yield reduction of approximately 0.1% after a year of operation.« less

  20. Measurement of radiation damage of water-based liquid scintillator and liquid scintillator

    SciTech Connect

    Bignell, L. J.; Diwan, M. V.; Hans, S.; Jaffe, D. E.; Rosero, R.; Vigdor, S.; Viren, B.; Worcester, E.; Yeh, M.; Zhang, C.

    2015-10-19

    Liquid scintillating phantoms have been proposed as a means to perform real-time 3D dosimetry for proton therapy treatment plan verification. We have studied what effect radiation damage to the scintillator will have upon this application. We have performed measurements of the degradation of the light yield and optical attenuation length of liquid scintillator and water-based liquid scintillator after irradiation by 201 MeV proton beams that deposited doses of approximately 52 Gy, 300 Gy, and 800 Gy in the scintillator. Liquid scintillator and water-based liquid scintillator (composed of 5% scintillating phase) exhibit light yield reductions of 1.74 ± 0.55 % and 1.31 ± 0.59 % after ≈ 800 Gy of proton dose, respectively. Some increased optical attenuation was observed in the irradiated samples, the measured reduction to the light yield is also due to damage to the scintillation light production. Based on our results and conservative estimates of the expected dose in a clinical context, a scintillating phantom used for proton therapy treatment plan verification would exhibit a systematic light yield reduction of approximately 0.1% after a year of operation.

  1. A Monte Carlo investigation of Swank noise for thick, segmented, crystalline scintillators for radiotherapy imaging

    PubMed Central

    Wang, Yi; Antonuk, Larry E.; El-Mohri, Youcef; Zhao, Qihua

    2009-01-01

    Thick, segmented scintillating detectors, consisting of 2D matrices of scintillator crystals separated by optically opaque septal walls, hold considerable potential for significantly improving the performance of megavoltage (MV) active matrix, flat-panel imagers (AMFPIs). Initial simulation studies of the radiation transport properties of segmented detectors have indicated the possibility of significant improvement in DQE compared to conventional MV AMFPIs based on phosphor screen detectors. It is therefore interesting to investigate how the generation and transport of secondary optical photons affect the DQE performance of such segmented detectors. One effect that can degrade DQE performance is optical Swank noise (quantified by the optical Swank factor Iopt), which is induced by depth-dependent variations in optical gain. In this study, Monte Carlo simulations of radiation and optical transport have been used to examine Iopt and zero-frequency DQE for segmented CsI:Tl and BGO detectors at different thicknesses and element-to-element pitches. For these detectors, Iopt and DQE were studied as a function of various optical parameters, including absorption and scattering in the scintillator, absorption at the top reflector and septal walls, as well as scattering at the side surfaces of the scintillator crystals. The results indicate that Iopt and DQE are only weakly affected by absorption and scattering in the scintillator, as well as by absorption at the top reflector. However, in some cases, these metrics were found to be significantly degraded by absorption at the septal walls and scattering at the scintillator side surfaces. Moreover, such degradations are more significant for detectors with greater thickness or smaller element pitch. At 1.016 mm pitch and with optimized optical properties, 40 mm thick segmented CsI:Tl and BGO detectors are predicted to provide DQE values of ∼29% and 42%, corresponding to improvement by factors of ∼29 and 42, respectively

  2. Cryogenic phonon-scintillation detectors with PMT readout for rare event search experiments

    NASA Astrophysics Data System (ADS)

    Zhang, X.; Lin, J.; Mikhailik, V. B.; Kraus, H.

    2016-06-01

    Cryogenic phonon-scintillation detectors (CPSD) for rare event search experiments require reliable, efficient and robust photon detectors that can resolve individual photons in a scintillation event. We report on a cryogenic detector containing a scintillating crystal, equipped with an NTD-Ge phonon sensor and a photon detector based on a low-temperature photomultiplier tube (PMT) that is powered by a Cockcroft-Walton generator. Here we present results from the characterisation of two detector modules, one with CaWO4, the other with CaMoO4 as scintillator. The energy resolutions (FWHM) at 122.1 keV for the scintillation/PMT channel are 19.9% and 29.7% respectively for CaWO4 and CaMoO4 while the energy resolutions (FWHM) for the phonon channels are 2.17 keV (1.8%) and 0.97 keV (0.79%). These characteristics compare favourably with other CPSDs currently used in cryogenic rare-event search experiments. The detection module with PMT readout benefits from the implementation of a well-understood, reliable, and commercially available component and improved time resolution, while retaining the major advantages of conventional CPSD, such as high sensitivity, resolving power and discrimination ability.

  3. Investigation of radiation detection properties of CRY-018 and CRY-019 scintillators for medical imaging

    NASA Astrophysics Data System (ADS)

    Pani, R.; Colarieti-Tosti, M.; Cinti, M. N.; Polito, C.; Trigila, C.; Ridolfi, S.

    2016-09-01

    During the last years the research for new scintillation crystals has been crucial for the improvement of imaging performance in nuclear medicine applications. Crytur company has recently released two new scintillators named CRY-018 and CRY-019 which are non hygroscopic, have short decay time and low refraction index. They represent the ideal candidates to substitute NaI:Tl and BGO crystals in future PET ad SPECT applications. The purpose of this work is to characterize this unknown crystals, look for possible applications in imaging for nuclear medicine. The results of this work were compared with the results obtained with a LaBr3:ce scintillation crystal. This particular crystal is used as a comparison benchmark because of its strong linear pulse height uniformity response and high energy resolution. Measurements have been performed with a high count rate which is typical for medical applications. Irradiation of the crystals have been performed in three different geometries and in a photon energy range suitable with SPECT and PET applications. The experimental results identify the CRY-018 as an Yttrium and Silicon mixture and the CRY-019 with as Lutetium and Silicon one. Moreover a light yield of about 45% of LaBr3 one, was obtained for both the CRY-018 and CRY-019. This is one of the higher light yield between most of the scintillation crystals usually used in nuclear medicine. Both crystals are characterized by a non-proportionality in the pulse height linearity response. Energy resolutions of 7.4% for CRY-018 and 8.4% for CRY-019 at 661 keV, have been measured. The intrinsic component of the energy resolution has been esteemed for all three scintillators. An intrinsic detection efficiency of about 45% at 122 keV for CRY-018 and 14% at 661 keV for CRY-019 has been measured. Compared with LaBr3:Ce efficiency, which is highly deteriorated by the coating required by the hygroscopicity, CRY-018 and CRY-019 are really interesting considering that these two samples

  4. Scintillation Breakdowns in Chip Tantalum Capacitors

    NASA Technical Reports Server (NTRS)

    Teverovsky, Alexander

    2008-01-01

    Scintillations in solid tantalum capacitors are momentarily local breakdowns terminated by a self-healing or conversion to a high-resistive state of the manganese oxide cathode. This conversion effectively caps the defective area of the tantalum pentoxide dielectric and prevents short-circuit failures. Typically, this type of breakdown has no immediate catastrophic consequences and is often considered as nuisance rather than a failure. Scintillation breakdowns likely do not affect failures of parts under surge current conditions, and so-called "proofing" of tantalum chip capacitors, which is a controllable exposure of the part after soldering to voltages slightly higher than the operating voltage to verify that possible scintillations are self-healed, has been shown to improve the quality of the parts. However, no in-depth studies of the effect of scintillations on reliability of tantalum capacitors have been performed so far. KEMET is using scintillation breakdown testing as a tool for assessing process improvements and to compare quality of different manufacturing lots. Nevertheless, the relationship between failures and scintillation breakdowns is not clear, and this test is not considered as suitable for lot acceptance testing. In this work, scintillation breakdowns in different military-graded and commercial tantalum capacitors were characterized and related to the rated voltages and to life test failures. A model for assessment of times to failure, based on distributions of breakdown voltages, and accelerating factors of life testing are discussed.

  5. Equatorial scintillations: advances since ISEA-6

    SciTech Connect

    Not Available

    1985-01-01

    Our understanding of the morphology of equatorial scintillations has advanced due to more intensive observations at the equatorial anomaly locations in the different longitude zones. The unmistakable effect of the sunspot cycle in controlling irregularity belt width and electron concentration responsible for strong scintillation in the controlling the magnitude of scintillations has been recognized by interpreting scintillation observations inthe light of realistic models of total electron content at various longitudes. A hypothesis based on the alignment of the solar terminator with the geomagnetic flux tubes as an indicator of enhanced scintillation occurrence and another based on the influence of a transequatorial thermospheric neutral wind have been postulated to describe the observed longitudinal variation. A distinct class of equatorial irregularities known as the bottomside sinusoidal (BSS) type was identified. These irregularities occur in very large patches, sometimes in excess of several thousand kilometers in the E-W direction and are associated with frequency spread on ionograms. Scintillations caused by such irregularities exist only in the VHF band, exhibit Fresnel oscillations in intensity spectra and are found to give rise to extremely long durations (approx. several hours) of uninterrrupted scintillations.

  6. Scintillation counter with WLS fiber readout

    NASA Astrophysics Data System (ADS)

    Bukin, D. A.; Druzhinin, V. P.; Golubev, V. B.; Serednyakov, S. I.

    1997-02-01

    The parameters of a cylindrical scintillation counter of 126 mm in diameter and 370 mm in length with wavelength shifter (WLS) fiber readout are presented. The fibers are glued into machined grooves along the scintillator. Light from both ends of the WLS fibers is transmitted to separate photomultipliers by 1 m long clear optical fibers. The average total signal, collected from both sides of the counter is equivalent to 8 photoelectrons per minimum ionizing particle. The described cylindrical scintillation counter is a part of inner system of collider detector SND.

  7. Scintillating Track Image Camera-SCITIC

    NASA Astrophysics Data System (ADS)

    Sato, Akira; Asai, Jyunkichi; Ieiri, Masaharu; Iwata, Soma; Kadowaki, Tetsuhito; Kurosawa, Maki; Nagae, Tomohumi; Nakai, Kozi

    2004-04-01

    A new type of track detector, scintillating track image camera (SCITIC) has been developed. Scintillating track images of particles in a scintillator are focused by an optical lens system on a photocathode on image intesifier tube (IIT). The image signals are amplified by an IIT-cascade and stored by a CCD camera. The performance of the detector has been tested with cosmic-ray muons and with pion- and proton-beams from the KEK 12-GeV proton synchrotron. Data of the test experiments have shown promising features of SCITIC as a triggerable track detector with a variety of possibilities.

  8. Measurement of light emission in scintillation vials

    SciTech Connect

    Duran Ramiro, M. Teresa; Garcia-Torano, Eduardo

    2005-09-15

    The efficiency and energy resolution of liquid scintillation counting (LSC) systems are strongly dependent on the optical characteristics of scintillators, vials, and reflectors. This article presents the results of measurements of the light-emission profile of scintillation vials. Two measurement techniques, autoradiographs and direct measurements with a photomultiplier tube, have been used to obtain light-emission distribution for standard vials of glass, etched glass and polyethylene. Results obtained with both techniques are in good agreement. For the first time, the effect of the meniscus in terms of light contribution has been numerically estimated. These results can help design LSC systems that are more efficient in terms of light collection.

  9. Advanced plastic scintillators for fast neutron discrimination

    SciTech Connect

    Feng, Patrick L; Anstey, Mitchell; Doty, F. Patrick; Mengesha, Wondwosen

    2014-09-01

    The present work addresses the need for solid-state, fast neutron discriminating scintillators that possess higher light yields and faster decay kinetics than existing organic scintillators. These respective attributes are of critical importance for improving the gamma-rejection capabilities and increasing the neutron discrimination performance under high-rate conditions. Two key applications that will benefit from these improvements include large-volume passive detection scenarios as well as active interrogation search for special nuclear materials. Molecular design principles were employed throughout this work, resulting in synthetically tailored materials that possess the targeted scintillation properties.

  10. Large volume flow-through scintillating detector

    DOEpatents

    Gritzo, Russ E.; Fowler, Malcolm M.

    1995-01-01

    A large volume flow through radiation detector for use in large air flow situations such as incinerator stacks or building air systems comprises a plurality of flat plates made of a scintillating material arranged parallel to the air flow. Each scintillating plate has a light guide attached which transfers light generated inside the scintillating plate to an associated photomultiplier tube. The output of the photomultiplier tubes are connected to electronics which can record any radiation and provide an alarm if appropriate for the application.

  11. Radiopure ZnMoO{sub 4} scintillating bolometers for the LUMINEU double-beta experiment

    SciTech Connect

    Poda, D. V.; Chernyak, D. M.; Armengaud, E.; Boissière, T. de; Fourches, N.; Gerbier, G.; Gros, M.; Hervé, S.; Magnier, P.; Navick, X-F.; Nones, C.; Paul, B.; Penichot, Y.; Arnaud, Q.; Augier, C.; Benoît, A.; Cazes, A.; Censier, B.; Charlieux, F.; De Jesus, M. [IPNL, Université de Lyon, Université Lyon 1, CNRS and others

    2015-08-17

    The results of R&D of radiopure zinc molybdate (ZnMoO{sub 4}) based scintillating bolometers for the LUMINEU (Luminescent Underground Molybdenum Investigation for NEUtrino mass and nature) double-beta decay experiment are presented. A dedicated two-stage molybdenum purification technique (sublimation in vacuum and recrystallization from aqueous solutions) and an advanced directional solidification method (the low-thermal-gradient Czochralski technique) were utilized to produce high optical quality large mass (∼1 kg) ZnMoO{sub 4} crystal boules and first {sup 100}Mo (99.5%) enriched Zn{sup 100}MoO{sub 4} crystal scintillator (mass of ∼0.2 kg). Scintillating bolometers based on ZnMoO{sub 4} (≈ 0.33 kg) and Zn{sup 100}MoO{sub 4} (≈ 0.06 kg) scintillation elements and high purity Ge wafers were tested in the EDELWEISS set-up at the Modane Underground Laboratory (France). Long term low temperature tests demonstrate excellent detectors’ performance and effectiveness of the purification and solidification procedures for the achievement of high radiopurity of the material, in particular with a bulk activity of {sup 228}Th and {sup 226}Ra below 4 µBq/kg. The adopted protocol was used to produce for the first time a large volume Zn{sup 100}MoO{sub 4} crystal scintillator (mass of ∼1.4 kg, {sup 100}Mo enrichment is 99.5%) to search for neutrinoless double-beta decay of {sup 100}Mo in the framework of the LUMINEU project.

  12. ZnWO4 anisotropic scintillator for Dark Matter investigation with the directionality technique

    NASA Astrophysics Data System (ADS)

    Bernabei, R.; Belli, P.; Cappella, F.; Caracciolo, V.; Cerulli, R.; Danevich, F. A.; d'Angelo, A.; Di Marco, A.; Incicchitti, A.; Mokina, V. M.; Poda, D. V.; Polischuk, O. G.; Taruggi, C.; Tretyak, V. I.

    2017-03-01

    The ZnWO4 crystal scintillator has unique features that make it very promising to realize a pioneering experiment to pursue Dark Matter investigation with the directionality technique. In particular in this detector the light output and the scintillation pulse shape for heavy particles (p, α, nuclear recoils) depend on the direction of the impinging particle with respect to the crystal axes, while the response to γ/β radiation is isotropic. The anisotropy of the light output can be considered to point out the presence in the diurnal counting rate of a Dark Matter signal produced by candidate particle inducing just nuclear recoils. In addition this crystal detector has also other important characteristics for a Dark Matter experiment: high light output, high level of radiopurity. In this paper the present performances of the developed ZnWO4 crystal scintillator will be summarized together with the possible future improvements. Some reachable sensitivities - under given assumptions - in the investigation of DM candidate particles with the directionality technique will also be addressed.

  13. Comparative studies of monoclinic and orthorhombic WO3 films used for hydrogen sensor fabrication on SiC crystal

    NASA Astrophysics Data System (ADS)

    Zuev, V. V.; Grigoriev, S. N.; Romanov, R. I.; Fominski, V. Y.; Volosova, M. A.; Demin, M. V.

    2016-09-01

    Amorphous WOx films were prepared on the SiC crystal by using two different methods, namely, reactive pulsed laser deposition (RPLD) and reactive deposition by ion sputtering (RDIS). After deposition, the WOx films were annealed in an air. The RISD film possessed a m-WO3 structure and consisted of closely packed microcrystals. Localized swelling of the films and micro-hills growth did not destroy dense crystal packing. RPLD film had layered β-WO3 structure with relatively smooth surface. Smoothness of the films were destroyed by localized swelling and the micro-openings formation was observed. Comparative study of m-WO3/SiC, Pt/m-WO3/SiC, and P-WO3/SiC samples shows that structural characteristics of the WO3 films strongly influence on the voltage/current response as well as on the rate of current growth during H2 detection at elevated temperatures.

  14. Research and Development of Scintillation fiber Trackers

    SciTech Connect

    Kobayashi, A.; ITO, H.; Kawai, H.; Kodama, S.; Kaneko, N.; Han, S.

    2015-07-01

    We are developing the scintillation fiber trackers. This detector is consist of 0.5 mm diameter scintillation fibers and PPDs. This detector has the doughnut shape with outer diameter of 50 cm and inner diameter of 10 cm and thickness of 2 mm. The position resolution is 70 μm. There are no ineffective area. And the cost is several million yen. (authors)

  15. Liquid scintillators for optical fiber applications

    DOEpatents

    Franks, Larry A.; Lutz, Stephen S.

    1982-01-01

    A multicomponent liquid scintillator solution for use as a radiation-to-light converter in conjunction with a fiber optic transmission system. The scintillator includes a quantity of 1, 2, 4, 5, 3H, 6H, 1 OH, tetrahydro-8-trifluoromethyl (1) benzopyrano (9, 9a, 1-gh) quinolizin-10-one (Coumarin) as a solute in a fluor solvent such as benzyl alcohol or pseudo-cumene. The use of BIBUQ as an additional or primary solute is also disclosed.

  16. Liquid scintillators for optical fiber applications

    SciTech Connect

    Franks, L.A.; Lutz, S.S.

    1982-11-16

    A multicomponent liquid scintillator solution for use as a radiation-to-light converter in conjunction with a fiber optic transmission system. The scintillator includes a quantity of 1, 2 , 4, 5, 3H, 6H, 1 OH, tetrahydro-8-trifluoromethyl (1) benzopyrano (9, 9a, 1-gh) quinolizin-10-one (Coumarin) as a solute in a fluor solvent such as benzyl alcohol or pseudocumene. The use of bibuq as an additional or primary solute is also disclosed.

  17. Ternary liquid scintillator for optical fiber applications

    DOEpatents

    Franks, Larry A.; Lutz, Stephen S.

    1982-01-01

    A multicomponent liquid scintillator solution for use as a radiation-to-light converter in conjunction with a fiber optic transmission system. The scintillator includes a quantity of 5-amino-9-diethylaminobenz (a) phenoxazonium nitrate (Nile Blue Nitrate) as a solute in a fluor solvent such as benzyl alcohol. The use of PPD as an additional solute is also disclosed. The system is controllable by addition of a suitable quenching agent, such as phenol.

  18. Current status on plastic scintillators modifications.

    PubMed

    Bertrand, Guillaume H V; Hamel, Matthieu; Sguerra, Fabien

    2014-11-24

    Recent developments of plastic scintillators are reviewed, from 2000 to March 2014, distributed in two different chapters. First chapter deals with the chemical modifications of the polymer backbone, whereas modifications of the fluorescent probe are presented in the second chapter. All examples are provided with the scope of detection of various radiation particles. The main characteristics of these newly created scintillators and their detection properties are given.

  19. Real-time volumetric scintillation dosimetry

    NASA Astrophysics Data System (ADS)

    Beddar, S.

    2015-01-01

    The goal of this brief review is to review the current status of real-time 3D scintillation dosimetry and what has been done so far in this area. The basic concept is to use a large volume of a scintillator material (liquid or solid) to measure or image the dose distributions from external radiation therapy (RT) beams in three dimensions. In this configuration, the scintillator material fulfills the dual role of being the detector and the phantom material in which the measurements are being performed. In this case, dose perturbations caused by the introduction of a detector within a phantom will not be at issue. All the detector configurations that have been conceived to date used a Charge-Coupled Device (CCD) camera to measure the light produced within the scintillator. In order to accurately measure the scintillation light, one must correct for various optical artefacts that arise as the light propagates from the scintillating centers through the optical chain to the CCD chip. Quenching, defined in its simplest form as a nonlinear response to high-linear energy transfer (LET) charged particles, is one of the disadvantages when such systems are used to measure the absorbed dose from high-LET particles such protons. However, correction methods that restore the linear dose response through the whole proton range have been proven to be effective for both liquid and plastic scintillators. Volumetric scintillation dosimetry has the potential to provide fast, high-resolution and accurate 3D imaging of RT dose distributions. Further research is warranted to optimize the necessary image reconstruction methods and optical corrections needed to achieve its full potential.

  20. Multi-GNSS for Ionospheric Scintillation Studies

    NASA Astrophysics Data System (ADS)

    Morton, Y.

    2015-12-01

    GNSS have been widely used for ionospheric monitoring. We anticipate over 160 GNSS satellites broadcasting 400 signals by 2023, nearly double the number today. With their well-defined signal structures, high spatial density and spectral diversity, GNSS offers low cost and distributed passive sensing of ionosphere effects. There are, however, many challenges to utilize GNSS resources to characterize and forecast ionospheric scintillation. Originally intended for navigation purposes, GNSS receivers are designed to filter out nuisance effects due to ionosphere effects. GNSS measurements are plagued with errors from multipath, oscillator jitters, processing artifacts, and neutral atmosphere effects. Strong scintillation events are often characterized by turbulent structures in ionosphere, causing simultaneous deep amplitude fading and abrupt carrier phase changes. The combined weak signal and high carrier dynamics imposes conflicting requirements for GNSS receiver design. Therefore, GNSS receivers often experience cycle slips and loss of lock of signals during strong scintillation events. High quality, raw GNSS signals bearing space weather signatures and robust receiver algorithms designed to capture these signatures are needed in order for GNSS to be a reliable and useful agent for scintillation monitoring and forecasting. Our event-driven, reconfigurable data collection system is designed to achieve this purpose. To date, our global network has collected ~150TB of raw GNSS data during space weather events. A suite of novel receiver processing algorithms has been developed by exploitating GNSS spatial, frequency, temporal, and constellation diversity to process signals experiencing challenging scintillation impact. The algorithms and data have advanced our understanding of scintillation impact on GNSS, lead to more robust receiver technologies, and enabled high spatial and temporal resolution depiction of ionosphere responses to solar and geomagnetic conditions. This

  1. A flexible scintillation light apparatus for rare event searches

    NASA Astrophysics Data System (ADS)

    Bonvicini, V.; Capelli, S.; Cremonesi, O.; Cucciati, G.; Gironi, L.; Pavan, M.; Previtali, E.; Sisti, M.

    2014-11-01

    Compelling experimental evidences of neutrino oscillations and their implication that neutrinos are massive particles have given neutrinoless double beta decay () a central role in astroparticle physics. In fact, the discovery of this elusive decay would be a major breakthrough, unveiling that neutrino and antineutrino are the same particle and that the lepton number is not conserved. It would also impact our efforts to establish the absolute neutrino mass scale and, ultimately, understand elementary particle interaction unification. All current experimental programs to search for are facing with the technical and financial challenge of increasing the experimental mass while maintaining incredibly low levels of spurious background. The new concept described in this paper could be the answer which combines all the features of an ideal experiment: energy resolution, low cost mass scalability, isotope choice flexibility and many powerful handles to make the background negligible. The proposed technology is based on the use of arrays of silicon detectors cooled to 120 K to optimize the collection of the scintillation light emitted by ultra-pure crystals. It is shown that with a 54 kg array of natural CaMoO scintillation detectors of this type it is possible to yield a competitive sensitivity on the half-life of the of Mo as high as years in only 1 year of data taking. The same array made of CaMoO scintillation detectors (to get rid of the continuous background coming from the two neutrino double beta decay of Ca) will instead be capable of achieving the remarkable sensitivity of years on the half-life of Mo in only 1 year of measurement.

  2. Validating the use of scintillation proxies to study ionospheric scintillation over the Ugandan region

    NASA Astrophysics Data System (ADS)

    Amabayo, Emirant B.; Jurua, Edward; Cilliers, Pierre J.

    2015-06-01

    In this study, we compare the standard scintillation indices (S4 and σΦ) from a SCINDA receiver with scintillation proxies (S4p and | sDPR |) derived from two IGS GPS receivers. Amplitude (S4) and phase (σΦ) scintillation data were obtained from the SCINDA installed at Makerere University (0.34°N, 32.57°E). The corresponding amplitude (S4p) and phase (| sDPR |) scintillation proxies were derived from data archived by IGS GPS receivers installed at Entebbe (0.04°N, 32.44°E) and Mbarara (0.60°S, 30.74°E). The results show that for most of the cases analysed in this study, σΦ and | sDPR | are in agreement. Amplitude scintillation occurrence estimated using the S4p are fairly consistent with the standard S4, mainly between 17:00 UT and 21:00 UT, despite a few cases of over and under estimation of scintillation levels by S4p. Correlation coefficients between σΦ and the | sDPR | proxy revealed positive correlation. Generally, S4p and S4 exhibits both moderate and strong positive correlation. TEC depletions associated with equatorial plasma bubbles are proposed as the cause of the observed scintillation over the region. These equatorial plasma bubbles were evident along the ray paths to satellites with PRN 2, 15, 27 and 11 as observed from MBAR and EBBE. In addition to equatorial plasma bubbles, atmospheric gravity waves with periods similar to those of large scale traveling ionospheric disturbances were also observed as one of the mechanisms for scintillation occurrence. The outcome of this study implies that GPS derived scintillation proxies can be used to quantify scintillation levels in the absence of standard scintillation data in the equatorial regions.

  3. Development of a Li2MoO4 scintillating bolometer for low background physics

    NASA Astrophysics Data System (ADS)

    Cardani, L.; Casali, N.; Nagorny, S.; Pattavina, L.; Piperno, G.; Barinova, O. P.; Beeman, J. W.; Bellini, F.; Danevich, F. A.; Di Domizio, S.; Gironi, L.; Kirsanova, S. V.; Orio, F.; Pessina, G.; Pirro, S.; Rusconi, C.; Tomei, C.; Tretyak, V. I.; Vignati, M.

    2013-10-01

    We present the performance of a 33 g Li2MoO4 crystal working as a scintillating bolometer. The crystal was tested for more than 400 h in a dilution refrigerator installed in the underground laboratory of Laboratori Nazionali del Gran Sasso (Italy). This compound shows promising features in the frame of neutron detection, dark matter search (solar axions) and neutrinoless double-beta decay physics. Low temperature scintillating properties were investigated by means of different α, β/γ and neutron sources, and for the first time the Light Yield for different types of interacting particle is estimated. The detector shows great ability of tagging fast neutron interactions and high intrinsic radiopurity levels ( < 90 μBq/kg for 238U and < 110 μBq/kg for 232Th).

  4. Performance of a prototype active veto system using liquid scintillator for a dark matter search experiment

    NASA Astrophysics Data System (ADS)

    Park, J. S.; Adhikari, P.; Adhikari, G.; Oh, S. Y.; Kim, N. Y.; Kim, Y. D.; Ha, C.; Park, K. S.; Lee, H. S.; Jeon, E. J.

    2017-04-01

    We report the performance of an active veto system using a liquid scintillator with NaI(Tl) crystals for use in a dark matter search experiment. When a NaI(Tl) crystal is immersed in the prototype detector, the detector tags 48% of the internal 40K background in the 0-10 keV energy region. We also determined the tagging efficiency for events at 6-20 keV as 26.5±1.7% of the total events, which corresponds to 0.76±0.04 events/keV/kg/day. According to a simulation, approximately 60% of the background events from U, Th, and K radioisotopes in photomultiplier tubes are tagged at energies of 0-10 keV. Full shielding with a 40-cm-thick liquid scintillator can increase the tagging efficiency for both the internal 40K and external background to approximately 80%.

  5. Hybrid metal organic scintillator materials system and particle detector

    DOEpatents

    Bauer, Christina A.; Allendorf, Mark D.; Doty, F. Patrick; Simmons, Blake A.

    2011-07-26

    We describe the preparation and characterization of two zinc hybrid luminescent structures based on the flexible and emissive linker molecule, trans-(4-R,4'-R') stilbene, where R and R' are mono- or poly-coordinating groups, which retain their luminescence within these solid materials. For example, reaction of trans-4,4'-stilbenedicarboxylic acid and zinc nitrate in the solvent dimethylformamide (DMF) yielded a dense 2-D network featuring zinc in both octahedral and tetrahedral coordination environments connected by trans-stilbene links. Similar reaction in diethylformamide (DEF) at higher temperatures resulted in a porous, 3-D framework structure consisting of two interpenetrating cubic lattices, each featuring basic to zinc carboxylate vertices joined by trans-stilbene, analogous to the isoreticular MOF (IRMOF) series. We demonstrate that the optical properties of both embodiments correlate directly with the local ligand environments observed in the crystal structures. We further demonstrate that these materials produce high luminescent response to proton radiation and high radiation tolerance relative to prior scintillators. These features can be used to create sophisticated scintillating detection sensors.

  6. Effect of Li+ ions co-doping on luminescence, scintillation properties and defects characteristics of LuAG:Ce ceramics

    NASA Astrophysics Data System (ADS)

    Liu, Shuping; Feng, Xiqi; Mares, Jiri A.; Babin, Vladimir; Hu, Chen; Kou, Huamin; D'Ambrosio, Carmelo; Li, Jiang; Pan, Yubai; Nikl, Martin

    2017-02-01

    Monovalent Li+ codoped Lu3Al5O12:Ce (LuAG:Ce) optical ceramics were fabricated by solid state reaction method and further optimized by an air-annealing process. Optical absorption, radioluminescence spectra and scintillation properties such as light yield, scintillation decay times and afterglow were measured and compared with those of the Li+ free LuAG:Ce ceramic and the commercial LuAG:Ce single crystal samples. Positive effect of Li+ codopant consists mainly in the significant increase of scintillation light yield, acceleration of scintillation decay as well as the decrease of afterglow intensity. With 0.3% Li codoping, the obtained LuAG:Ce,Li ceramic displays a light yield of ∼29200 ph/MeV at 10 μs shaping time, higher than that of the LuAG:Ce single crystal and optical ceramic scintillators ever reported. The partial conversion of the stable Ce3+ to Ce4+ centers and the shallow and deep traps effect suppression by the Li+ codoping are discussed.

  7. Possible application of scintillation detectors with semiconductor PMT for cosmic-neutron and gamma-ray detection

    NASA Astrophysics Data System (ADS)

    Mokrousov, M. I.; Vostrukhin, A. A.; Karpushkina, N. E.; Malakhov, A. V.

    2016-09-01

    Solar system planets exploration and cosmic neutrons and gamma-ray flux research have been dynamically evolving for several decades. Different scintillation crystals are used for this purpose along with photo signal receivers, such as vacuum photomultiplier tubes (PMT). Many studies are being performed in order to provide alternative devices for photon signal capture: PIN-diodes,avalanche photodiodes, semiconductor silicon photomultipliers. We study the applicability of a silicon PMT in employing highresolution crystals in space applications.

  8. Detection of gamma-neutron radiation by solid-state scintillation detectors. Detection of gamma-neutron radiation by novel solid-state scintillation detectors

    SciTech Connect

    Ryzhikov, V.; Grinyov, B.; Piven, L.; Onyshchenko, G.; Sidletskiy, O.; Naydenov, S.; Pochet, T.; Smith, C.

    2015-07-01

    It is known that solid-state scintillators can be used for detection of both gamma radiation and neutron flux. In the past, neutron detection efficiencies of such solid-state scintillators did not exceed 5-7%. At the same time it is known that the detection efficiency of the gamma-neutron radiation characteristic of nuclear fissionable materials is by an order of magnitude higher than the efficiency of detection of neutron fluxes alone. Thus, an important objective is the creation of detection systems that are both highly efficient in gamma-neutron detection and also capable of exhibiting high gamma suppression for use in the role of detection of neutron radiation. In this work, we present the results of our experimental and theoretical studies on the detection efficiency of fast neutrons from a {sup 239}Pu-Be source by the heavy oxide scintillators BGO, GSO, CWO and ZWO, as well as ZnSe(Te, O). The most probable mechanism of fast neutron interaction with nuclei of heavy oxide scintillators is the inelastic scattering (n, n'γ) reaction. In our work, fast neutron detection efficiencies were determined by the method of internal counting of gamma-quanta that emerge in the scintillator from (n, n''γ) reactions on scintillator nuclei with the resulting gamma energies of ∼20-300 keV. The measured efficiency of neutron detection for the scintillation crystals we considered was ∼40-50 %. The present work included a detailed analysis of detection efficiency as a function of detector and area of the working surface, as well as a search for new ways to create larger-sized detectors of lower cost. As a result of our studies, we have found an unusual dependence of fast neutron detection efficiency upon thickness of the oxide scintillators. An explanation for this anomaly may involve the competition of two factors that accompany inelastic scattering on the heavy atomic nuclei. The transformation of the energy spectrum of neutrons involved in the (n, n'γ) reactions towards

  9. The Advanced Scintillator Compton Telescope (ASCOT) balloon project

    NASA Astrophysics Data System (ADS)

    Bloser, Peter F.; Sharma, Tejaswita; Legere, Jason S.; Bancroft, Christopher M.; McConnell, Mark L.; Ryan, James M.; Wright, Alex M.

    2016-07-01

    We describe a project to develop new medium-energy gamma-ray instrumentation by constructing and flying a balloon-borne Compton telescope using advanced scintillator materials combined with silicon photomultiplier readouts. There is a need in high-energy astronomy for a medium-energy gamma-ray mission covering the energy range from approximately 0.4 - 20 MeV to follow the success of the COMPTEL instrument on CGRO. We believe that directly building on the legacy of COMPTEL, using relatively robust, low-cost, off-the-shelf technologies, is the most promising path for such a mission. Fortunately, high-performance scintillators, such as Lanthanum Bromide (LaBr3), Cerium Bromide (CeBr3), and p-terphenyl, and compact readout devices, such as silicon photomultipliers (SiPMs), are already commercially available and capable of meeting this need. We have conducted two balloon flights of prototype instruments to test these technologies. The first, in 2011, demonstrated that a Compton telescope consisting of an liquid organic scintillator scattering layer and a LaBr3 calorimeter effectively rejects background under balloon-flight conditions, using time-of-flight (ToF) discrimination. The second, in 2014, showed that a telescope using an organic stilbene crystal scattering element and a LaBr3 calorimeter with SiPM readouts can achieve similar ToF performance. We are now constructing a much larger balloon instrument, an Advanced Scintillator Compton Telescope (ASCOT) with SiPM readout, with the goal of imaging the Crab Nebula at MeV energies in a one-day flight. We expect a 4σ detection up to 1 MeV in a single transit. We present calibration results of the first detector modules, and updated simulations of the balloon instrument sensitivity. If successful, this project will demonstrate that the energy, timing, and position resolution of this technology are sufficient to achieve an order of magnitude improvement in sensitivity in the mediumenergy gamma-ray band, were it to be

  10. A Depth-of-Interaction encoding method for SPECT monolithic scintillation detectors

    NASA Astrophysics Data System (ADS)

    Bettiol, M.; Preziosi, E.; Cinti, M. N.; Borrazzo, C.; Fabbri, A.; Cassano, B.; Polito, C.; Pellegrini, R.; Pani, R.

    2016-12-01

    The Depth of Interaction (DoI) discrimination of gamma-photons within scintillation crystals allows to improve imaging performance in PET scanners as well as in SPECT devices equipped with non-parallel collimators (e. g. pinhole ones). In previous works, the authors experimentally proved the efficiency of a DoI-encoding technique in case of a 20 mm-thick monolithic crystal PET module. For the thinner crystals commonly used in SPECT, DoI determination still remains a challenging goal. To this aim, in this work the authors have experimentally evaluated the DoI-encoding method on a 6 mm-thick monolithic LaBr3:Ce crystal. The results prove the efficiency and reliability of the proposed method. It indeed allows to discriminate the gamma photons interacting at the the top and the bottom of the crystal.

  11. Mg co-doping effects on Ce doped Y3(Ga,Al)5O12 scintillator

    NASA Astrophysics Data System (ADS)

    Kamada, Kei; Yamaji, Akihiro; Kurosawa, Shunsuke; Yokota, Yuui; Ohashi, Yuji; Yoshikawa, Akira

    2017-02-01

    Nonstoichiometric Lu3Al5+xO12 (x= 0.05, 0.15, 0.35, 0, -0.05, -0.15, -0.35) crystals were grown by the μ-PD method. Luminescence and scintillation properties such as absorption, excitation and emission spectra, light yield and decay time were evaluated. Expected anti-site defect related host emission have been observed in 250-420nm. Emission intensity was increased by increasing the nonstochiometry. The x=-0.35 sample showed the highest light yield of around 12000 photons/MeV and slowest scintillation decay time of 1.96μs.

  12. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    DOE PAGES

    Rusev, Gencho Yordanov; Jandel, Marian; Baramsai, Bayarbadrakh; ...

    2015-08-26

    Here, investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flightmore » spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.« less

  13. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    SciTech Connect

    Rusev, Gencho Yordanov; Jandel, Marian; Baramsai, Bayarbadrakh; Bond, Evelyn M.; Bredeweg, Todd Allen; Couture, Aaron Joseph; Daum, Jaimie Kay; Favalli, Andrea; Ianakiev, Kiril Dimitrov; Iliev, Metodi L.; Mosby, Shea Morgan; Roman, Audrey Rae; Springs, Rebecca Kristien; Ullmann, John Leonard; Walker, Carrie Lynn

    2015-08-26

    Here, investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  14. New concepts for scintillator/HgI[sub 2] gamma ray spectroscopy

    SciTech Connect

    Wang, Y.J.; Iwanczyk, J.S.; Patt, B.E. )

    1994-08-01

    The construction of a high energy resolution gamma ray detector consisting of a scintillator/mercuric iodide photodetector combination has been investigated. Several HgI[sub 2] photodetectors have been fabricated and tested with standard NIM electronics. The energy resolution of a scintillator/HgI[sub 2] pair was found to be 4.75%, full width at half maximum, for 662 keV [sup 137]Cs gamma ray photons. Of five detectors fabricated with the new technique, all produced resolutions better than 5.6% FWHM. This technology makes it possible to reliably produce high quality HgI[sub 2] photodetectors. New design concepts for the HgI[sub 2] photocell, including the transparent entrance electrode, detector geometry, and detector packaging, are described in the paper. Advantages of gamma ray spectrometers based upon crystal scintillators optically coupled to HgI[sub 2] photodetectors (in contrast to coupling the scintillators to the more conventional light sensors, i.e., photomultiplier tubes (PMTs)) include greater ruggedness, improved energy resolution, markedly smaller size and weight, reduced power, and insensitivity to magnetic field perturbations.

  15. High-efficiency fast scintillators for 'optical' soft x-ray arrays for laboratory plasma diagnostics

    SciTech Connect

    Delgado-Aparicio, L. F.; Stutman, D.; Tritz, K.; Vero, R.; Finkenthal, M.; Suliman, G.; Kaita, R.; Majeski, R.; Stratton, B.; Roquemore, L.; Tarrio, C

    2007-08-20

    Scintillator-based 'optical' soft x-ray (OSXR) arrays have been investigated as a replacement for the conventional silicon (Si)-based diode arrays used for imaging, tomographic reconstruction, magnetohydrodynamics, transport, and turbulence studies in magnetically confined fusion plasma research. An experimental survey among several scintillator candidates was performed, measuring the relative and absolute conversion efficiencies of soft x rays to visible light. Further investigations took into account glass and fiber-optic faceplates (FOPs) as substrates, and a thin aluminum foil(150 nm) to reflect the visible light emitted by the scintillator back to the optical detector.Columnar (crystal growth) thallium-doped cesium iodide (CsI:Tl) deposited on an FOP, was found to be the best candidate for the previously mentioned plasma diagnostics.Its luminescence decay time of the order of?1-10 {mu}s is thus suitable for the 10 {mu}s time resolution required for the development of scintillator-based SXR plasma diagnostics. A prototype eight channel OSXR array using CsI:Tl was designed, built,and compared to an absolute extreme ultraviolet diode counterpart: its operation on the National Spherical Torus Experiment showed a lower level of induced noise relative to the Si-based diode arrays, especially during neutral beam injection heated plasma discharges. The OSXR concept can also be implemented in less harsh environments for basic spectroscopic laboratory plasma diagnostics.

  16. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    NASA Astrophysics Data System (ADS)

    Rusev, G.; Jandel, M.; Baramsai, B.; Bond, E. M.; Bredeweg, T. A.; Couture, A.; Daum, J. K.; Favalli, A.; Ianakiev, K. D.; Iliev, M. L.; Mosby, S.; Roman, A. R.; Springs, R. K.; Ullmann, J. L.; Walker, C. L.

    2015-08-01

    Investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  17. Response of a lithium gadolinium borate scintillator in monoenergetic neutron fields.

    PubMed

    Williams, A M; Beeley, P A; Spyrou, N M

    2004-01-01

    Accurate estimation of neutron dose requires knowledge of the neutron energy distribution in the working environment. Existing neutron spectrometry systems, Bonner spheres for example, are large and bulky, and require long data acquisition times. A portable system that could indicate the approximate neutron energy spectrum in a short time would be extremely useful in radiation protection. A composite scintillator, consisting of lithium gadolinium borate crystals in a plastic scintillator matrix, produced by Photogenics is being tested for this purpose. A prototype device based on this scintillator and digital pulse processing electronics has been calibrated using quasi-monoenergetic neutron fields at the low-scatter facility of the UK National Physical Laboratory (NPL). Energies selected were 144, 250, 565, 1400, 2500 and 5000 keV, with correction for scattered neutrons being made using the shadow cone technique. Measurements were also made in the NPL thermal neutron field. Pulse distributions collected with the digitiser in capture-gated mode are presented, and detection efficiency and energy resolution derived. For comparison, neutron spectra were also collected using the commercially available Microspec N-Probe from Bubble Technology Industries, which consists of an NE213 scintillator and a 3He proportional counter.

  18. Rare isotope beam energy measurements and scintillator developments for ReA3

    NASA Astrophysics Data System (ADS)

    Lin, Ling-Ying

    respect to the acceleration RF clock. The time-of-flight system can provide beam energy information with precision of <0.1%. Scintillators are widely used to reliably measure beam profiles and beam distributions. At low energies, scintillator-based diagnostic devices are more problematic because of their fast light yield degradation under ion bombardment. The degradation of the scintillation yield of single crystal YAG: Ce under He+ irradiation at low energies between 28 and 58 keV has been systematically studied. The scintillator was irradiated at the rare isotope ReAccelerator (ReA) facility. The scintillation emission is attributed to its rapid 5d-4f transition of Ce3+ ions. As the bombardment time increases, an exponential decay of the light output is observed due to the induced radiation damage of the crystal lattice. The decrease of the experimentally observed light yield as a function of particle fluence is found to be in fair agreement with the Birks model. Analysis indicates that the damage cross section of scintillation centers slightly decreases with the ion energy. The scintillator degrades slower under higher-energy irradiation. In order to investigate scintillation degradation over a wide range of irradiation energies and scintillator materials, the scintillation processes for KBr, YAG:Ce, CaF2:Eu and CsI:Tl crystals under H2 + irradiation in the energy range of 600-2150 keV/u have been investigated. The data indicates that YAG:Ce and CsI:Tl can maintain stable luminescence under continuous ion bombardment for at least a total fluence of 1.8x10 12 ions/mm2. On the other hand, the luminescence of CaF2:Eu shows a rapid initial decay but then maintains a nearly constant luminescence yield. The extraordinary scintillation response of KBr is initially enhanced under ion bombardment, approaches a maximum, and then eventually decays. The scintillation efficiency of the CsI:Tl scintillator is superior to the other materials. The low-energy H2+ bombardment (25 ke

  19. Isotopic response with small scintillator based gamma-ray spectrometers

    DOEpatents

    Madden, Norman W [Sparks, NV; Goulding, Frederick S [Lafayette, CA; Asztalos, Stephen J [Oakland, CA

    2012-01-24

    The intrinsic background of a gamma ray spectrometer is significantly reduced by surrounding the scintillator with a second scintillator. This second (external) scintillator surrounds the first scintillator and has an opening of approximately the same diameter as the smaller central scintillator in the forward direction. The second scintillator is selected to have a higher atomic number, and thus has a larger probability for a Compton scattering interaction than within the inner region. Scattering events that are essentially simultaneous in coincidence to the first and second scintillators, from an electronics perspective, are precluded electronically from the data stream. Thus, only gamma-rays that are wholly contained in the smaller central scintillator are used for analytic purposes.

  20. Quenching factor for alpha particles in ZnSe scintillating bolometers

    NASA Astrophysics Data System (ADS)

    Nagorny, S.; Cardani, L.; Casali, N.; Dafinei, I.; Pagnanini, L.; Pattavina, L.; Pirro, S.; Schaeffner, K.

    2017-02-01

    In the framework of the CUPID-0 experiment, a numbers of ZnSe single crystals were produced and subjected to different thermal treatments, and later tested as cryogenic scintillating bolometers. We have found that a specific thermal treatment (24 hours under argon atmosphere at 900 °C) has a strong impact on some properties of ZnSe crystals (amplitude of signal, light yield, specific resistivity) and most interestingly, changes the quenching factor for alpha particles from values > 1 to values < 1. Thus such thermal treatment opens the possibility to modify this experimental parameter for a various applications.

  1. Impact of precursor purity on optical properties and radiation detection of CsI:Tl scintillators

    NASA Astrophysics Data System (ADS)

    Saengkaew, Phannee; Sanorpim, Sakuntam; Jitpukdee, Manit; Cheewajaroen, Kulthawat; Yenchai, Chadet; Thong-aram, Decho; Yordsri, Visittapong; Thanachayanont, Chanchana; Nuntawong, Noppadon

    2016-08-01

    Cesium iodide doped with thallium (CsI:Tl) crystals was grown to develop the gamma-ray detectors by using low-cost raw materials. Effect of impurities on optical properties and radiation detection performance was investigated. By a modified homemade Bridgman-Stockbarger technique, CsI:Tl samples were grown in two levels of CsI and TlI reactant materials, i.e., having as a very high purity of 99.999 % and a high purity of 99.9 %. XRD measurements indicate CsI:Tl crystals having a good quality with a dominant (110) plane. Having a cubic structure, a lattice constant of CsI crystals of 0.4574 nm and a crystallite size of 43.539 nm were obtained. From the lower-purity raw materials, calcite was found in an orange crystal with a lattice constant of 0.4560 nm and a crystallite size of 43.089 nm. By PL measurements, the optical properties of the CsI:Tl crystals were analyzed. ~540-nm-wavelength PL peak was observed from the colorless high-purity crystal, and ~600-nm-wavelength PL peak was observed from the orange crystal. The brighter PL emission was obtained from the orange crystals suggesting impurities. CsI:Tl surface morphology by SEM exhibited a smooth surface with some parallel crystal facets. For electrical properties of high-quality CsI:Tl crystals, the electrical resistances were 230 ± 16 MΩ in cross-sectional direction and 714 ± 136 MΩ in vertical direction with respect to more homogeneous crystal quality in cross-sectional direction than that in vertical direction. TEM measurement was applied to evaluate the microstructure of colorless CsI:Tl crystal with different patterns of a cubic structure. Both CsI:Tl crystals show good efficiencies and good resolutions. Maintaining the same electronic conditions and amplifications, the colorless CsI:Tl scintillators represented a higher detection efficiency at 122 keV of Co-57 of 78.4 % and the energy resolution of 23.3 % compared to the detection efficiency of 75.9 % and the energy resolution of 34.6 % of the orange

  2. ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy

    NASA Astrophysics Data System (ADS)

    Ji, J.; Colosimo, A. M.; Anwand, W.; Boatner, L. A.; Wagner, A.; Stepanov, P. S.; Trinh, T. T.; Liedke, M. O.; Krause-Rehberg, R.; Cowan, T. E.; Selim, F. A.

    2016-08-01

    The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials.

  3. ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy

    PubMed Central

    Ji, J.; Colosimo, A. M.; Anwand, W.; Boatner, L. A.; Wagner, A.; Stepanov, P. S.; Trinh, T. T.; Liedke, M. O.; Krause-Rehberg, R.; Cowan, T. E.; Selim, F. A.

    2016-01-01

    The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials. PMID:27550235

  4. ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy.

    PubMed

    Ji, J; Colosimo, A M; Anwand, W; Boatner, L A; Wagner, A; Stepanov, P S; Trinh, T T; Liedke, M O; Krause-Rehberg, R; Cowan, T E; Selim, F A

    2016-08-23

    The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials.

  5. Scintillating-glass-fiber neutron sensors

    NASA Astrophysics Data System (ADS)

    Abel, K. H.; Arthur, R. J.; Bliss, M.; Brite, D. W.; Brodzinski, R. L.; Craig, R. A.; Geelhood, B. D.; Goldman, D. S.; Griffin, J. W.; Perkins, R. W.; Reeder, P. L.; Richey, W. R.; Stahl, K. A.; Sunberg, D. S.; Warner, R. A.; Wogman, N. A.; Weber, M. J.

    1994-12-01

    Cerium-doped lithium-silicate glass fibers have been developed at Pacific Northwest Laboratory (PNL) for use as thermal neutron detectors. By using highly-enriched 6Li, these fibers efficiently capture thermal neutrons and produce scintillation light that can be detected at the ends of the fibers. Advantages of scintillating fibers over 3He or BF 3 proportional tubes include flexibility in geometric configuration, ruggedness in high-vibration environments, and less detector weight for the same neutron sensitivity. This paper describes the performance of these scintillating fibers with regard to count rates, pulse height spectra, absolute efficiencies, and neutron/gamma discrimination. Fibers with light transmission lengths ( {1}/{e}) of greater than 2 m have been produced at PNL. Neutron sensors in fiber form allow development of a variety of neutron detectors packaged in previously unavailable configurations. Brief descriptions of some of the devices already produced are included to illustrate these possibilities.

  6. Current trends in scintillator detectors and materials

    SciTech Connect

    Moses, William W.

    2001-10-23

    The last decade has seen a renaissance in inorganic scintillator development for gamma ray detection. Lead tungstate (PbWO4) has been developed for high energy physics experiments, and possesses exceptionally high density and radiation hardness, albeit with low luminous efficiency. Lutetium orthosilicate or LSO (Lu2SiO5:Ce) possesses a unique combination of high luminous efficiency, high density, and reasonably short decay time, and is now incorporated in commercial positron emission tomography (PET) cameras. There have been advances in understanding the fundamental mechanisms that limit energy resolution, and several recently discovered materials (such as LaBr3:Ce) possess energy resolution that approaches that of direct solid state detectors. Finally, there are indications that a neglected class of scintillator materials that exhibit near band-edge fluorescence could provide scintillators with sub-nanosecond decay times and high luminescent efficiency.

  7. On the scintillation efficiency of carborane-loaded liquid scintillators for thermal neutron detection

    NASA Astrophysics Data System (ADS)

    Chang, Zheng; Okoye, Nkemakonam C.; Urffer, Matthew J.; Green, Alexander D.; Childs, Kyle E.; Miller, Laurence F.

    2015-01-01

    The scintillation efficiency in response to thermal neutrons was studied by loading different concentrations of carborane (0-8.5 wt%) and naphthalene (0 and 100 g/L) in five liquid organic scintillators. The sample was characterized in Pb and Cd shields under the irradiation of the thermal neutrons from a 252Cf source. A method was developed to extract the net neutron response from the pulse-height spectra. It was found that the order of scintillation efficiencies for both γ-rays and thermal neutrons is as follows: diisopropylnaphthalene>toluene (concentrated solutes)>toluene~pseudocumene~m-xylene. The quench constants, obtained by fitting the Stern-Volmer model to the plots of light output versus carborane concentration, are in the range of 0.35-1.4 M-1 for all the scintillators. The Birks factors, estimated using the specific energy loss profiles of the incident particles, are in the range of 9.3-14 mg cm-2 MeV-1 for all the samples. The light outputs are in the range of 63-86 keV electron equivalents (keVee) in response to thermal neutrons. Loading naphthalene generally promotes the scintillation efficiency of the scintillator with a benzene derivative solvent. Among all the scintillators tested, the diisopropylnaphthalene-based scintillator shows the highest scintillation efficiency, lowest Birks factor, and smallest quench constants. These properties are primarily attributed to the double fused benzene-ring structure of the solvent, which is more efficient to populate to the excited singlet state under ionizing radiation and to transfer the excitation energy to the fluorescent solutes.

  8. The design of the TASD (totally active scintillator detector) prototype

    SciTech Connect

    Mefodiev, A. V. Kudenko, Yu. G.

    2015-12-15

    Totally active and magnetic segmented scintillation neutrino detectors are developed for the nextgeneration accelerator neutrino experiments. Such detectors will incorporate scintillation modules with scintillation counters that form X and Y planes. A single counter is a 7 × 10 × 90 mm{sup 3} scintillation bar with gluedin wavelength-shifting fibers and micropixel avalanche photodiodes. The results of measurements of the parameters of these detectors are presented.

  9. Statistics of time averaged atmospheric scintillation

    SciTech Connect

    Stroud, P.

    1994-02-01

    A formulation has been constructed to recover the statistics of the moving average of the scintillation Strehl from a discrete set of measurements. A program of airborne atmospheric propagation measurements was analyzed to find the correlation function of the relative intensity over displaced propagation paths. The variance in continuous moving averages of the relative intensity was then found in terms of the correlation functions. An empirical formulation of the variance of the continuous moving average of the scintillation Strehl has been constructed. The resulting characterization of the variance of the finite time averaged Strehl ratios is being used to assess the performance of an airborne laser system.

  10. Plastic scintillator centrality detector for BRAHMS

    NASA Astrophysics Data System (ADS)

    Lee, Y. K.; Debbe, R.; Lee, J. H.; Ito, Hironori; Sanders, S. J.

    2004-01-01

    An array of 40 tiles of thin plastic scintillators is used to construct the outer layer of the charged particle multiplicity detector for the BRAHMS experiment at the Relativistic Heavy Ion Collider (RHIC). Each tile is a square with 12 cm long sides and 5 mm thickness. The light from each of the scintillators is collected by wavelength shifting fibers embedded on the periphery. The light collection is uniform within 5% over the tile with the edge effect limited to 4 mm along the edge. The response is found to be linear in the high-multiplicity environment at RHIC with Au+Au beams at s NN of 200 GeV.

  11. Quality study of the purified liquid scintillator

    NASA Astrophysics Data System (ADS)

    Konno, Y.; Nakajima, K.; Kibe, Y.

    2008-07-01

    We have been distilling the KamLAND liquid scintillator (LS) for the low energy solar neutrino observation. The distillation removes radioactive impurities from LS efficiently. We developed two types of high sensitivity radon detectors to monitor 222Rn contamination which causes a primary background source 210Pb. Their required sensitivity is several mBq/m3. The features and the measurement results of these detectors are presented. We also report the study of liquid scintillator properties after the distillation: attenuation length, light output and PPO density.

  12. Effects of radiation on scintillating fiber performance

    SciTech Connect

    Bauer, M.L.; Cohn, H.; Efremenko, Yu.; Gordeev, A.; Kamyshkov, Yu.; Onopienko, D.; Savin, S.; Shmakov, K.; Tarkovsky, E.; Young, K.G.; Carey, R.; Rothman, M.; Sulak, L.; Worstell, W.; Parr, H.

    1992-12-31

    Continued rapid improvements in formulations for scintillating fibers require the ability to parameterize and predict effects of radiation on detector performance. Experimental techniques necessary to obtain needed information and calculational procedures used in performing predications for hadron scintillating fiber calorimetry in the Superconducting Supercollider environment are described. The experimental techniques involve control of the testing environment, consideration of dose rate effects, and other factors. These calculations involve the behavior of particle showers in the detector, expected levels of radiation, and parameterization of the radiation effects. A summary of significant work is also presented.

  13. Effects of radiation on scintillating fiber performance

    SciTech Connect

    Young, K.G.; Bauer, M.L.; Cohn, H.; Efremenko, Yu.; Gordeev, A.; Kamyshkov, Yu.; Onopienko, D.; Savin, S.; Shmakov, K.; Tarkovsky, E. ); Carey, R.; Rothman, M.; Sulak, L.; Worstell, W. ); Paar, H. )

    1993-08-01

    Continued rapid improvements in formulations for scintillating fibers require the ability to parameterize and predict effects of radiation on detector performance. Experimental techniques necessary to obtain desired information and calculational procedures used in performing predictions for hadron scintillating fiber calorimetry in the Superconducting Supercollider environment are described. The experimental techniques involve control of the testing environment, consideration of dose rate effects, and other factors. The calculations involve the behavior of particle showers in the detector, expected levels of radiation, and parameterization of the radiation effects. A summary of significant work is also presented.

  14. Near-infrared scintillation of liquid argon

    SciTech Connect

    Alexander, T.; Escobar, C. O.; Lippincott, W. H.; Rubinov, P.

    2016-03-03

    Since the 1970s it has been known that noble gases scintillate in the near infrared (NIR) region of the spectrum (0.7 $\\mu$m < $\\lambda$; < 1.5$\\mu$m). More controversial has been the question of the NIR light yield for condensed noble gases. We first present the motivation for using the NIR scintillation in liquid argon detectors, then briefly review early as well as more recent efforts and finally show encouraging preliminary results of a test performed at Fermilab.

  15. The homestake surface-underground scintillations: Description

    NASA Technical Reports Server (NTRS)

    Cherry, M. L.; Corbato, S.; Daily, T.; Fenyves, E. J.; Kieda, D.; Lande, K.; Lee, C. K.

    1985-01-01

    Two new detectors are currently under construction at the Homestake Gold Mine a 140-ton Large Area Scintillation Detector (LASD) with an upper surface area of 130 square meters, a geometry factor (for an isotropic flux) of 1200 square meters, sr, and a depth of 4200 m.w.e.; and a surface air shower array consisting of 100 scintillator elements, each 3 square meters, spanning an area of approximately square kilometers. Underground, half of the LASD is currently running and collecting muon data; on the surface, the first section of the air shower array will begin operation in the spring of 1985. The detectors and their capabilities are described.

  16. Plastic scintillators modifications for a selective radiation detection

    SciTech Connect

    Hamel, Matthieu; Bertrand, Guillaume H.V.; Carrel, Frederick; Coulon, Romain; Dumazert, Jonathan; Montbarbon, Eva; Sguerra, Fabien

    2015-07-01

    Recent developments of plastic scintillators are reviewed, from January 2000 to June 2015. All examples are distributed into the main application, i.e. how the plastic scintillator was modified to enhance the detection towards a given radiation particle. The main characteristics of these newly created scintillators and their detection properties are given. (authors)

  17. New liquid scintillators for fiber-optic applications

    SciTech Connect

    Lutz, S.S.; Franks, L.A.; Flournoy, J.M.; Lyons, P.B.

    1981-01-01

    New long-wavelength-emitting, high-speed, liquid scintillators have been developed and tailored specifically for plasma diagnostic experiments employing fiber optics. These scintillators offer significant advantages over commercially available plastic scintillators in terms of sensitivity and bandwidth. FWHM response times as fast as 350 ps have been measured. Emission spectra, time response data, and relative sensitivity information are presented.

  18. Upconverting nanoparticles for optimizing scintillator based detection systems

    DOEpatents

    Kross, Brian; McKisson, John E; McKisson, John; Weisenberger, Andrew; Xi, Wenze; Zom, Carl

    2013-09-17

    An upconverting device for a scintillation detection system is provided. The detection system comprises a scintillator material, a sensor, a light transmission path between the scintillator material and the sensor, and a plurality of upconverting nanoparticles particles positioned in the light transmission path.

  19. Sub-200 ps CRT in monolithic scintillator PET detectors using digital SiPM arrays and maximum likelihood interaction time estimation.

    PubMed

    van Dam, Herman T; Borghi, Giacomo; Seifert, Stefan; Schaart, Dennis R

    2013-05-21

    Digital silicon photomultiplier (dSiPM) arrays have favorable characteristics for application in monolithic scintillator detectors for time-of-flight positron emission tomography (PET). To fully exploit these benefits, a maximum likelihood interaction time estimation (MLITE) method was developed to derive the time of interaction from the multiple time stamps obtained per scintillation event. MLITE was compared to several deterministic methods. Timing measurements were performed with monolithic scintillator detectors based on novel dSiPM arrays and LSO:Ce,0.2%Ca crystals of 16 × 16 × 10 mm(3), 16 × 16 × 20 mm(3), 24 × 24 × 10 mm(3), and 24 × 24 × 20 mm(3). The best coincidence resolving times (CRTs) for pairs of identical detectors were obtained with MLITE and measured 157 ps, 185 ps, 161 ps, and 184 ps full-width-at-half-maximum (FWHM), respectively. For comparison, a small reference detector, consisting of a 3 × 3 × 5 mm(3) LSO:Ce,0.2%Ca crystal coupled to a single pixel of a dSiPM array, was measured to have a CRT as low as 120 ps FWHM. The results of this work indicate that the influence of the optical transport of the scintillation photons on the timing performance of monolithic scintillator detectors can at least partially be corrected for by utilizing the information contained in the spatio-temporal distribution of the collection of time stamps registered per scintillation event.

  20. Latest advances in large diameter SrI:Eu and CLYC:Ce scintillators for isotope identification

    SciTech Connect

    Hawrami, Rastgo; Hines, C; Abselem, I; Biteman, V; Vaghini, J; Glodo, J.; O’Dougherty, P; Shah, Kanai; Cherepy, Nerine; Payne, Stephen A.; Burger, Arnold; Boatner, Lynn A

    2012-01-01

    Scintillator crystal detectors form the basis for many radiation detection devices. Therefore, a search for high light yield single crystal scintillators with improved energy resolution, large volume, and the potential for low cost, is an ongoing process that has increased in recent years due to a large demand in the area of nuclear isotope identification. Alkaline earth halides, elpasolites and rare earth halides are very interesting because many compositions from these crystal families provide efficient Ce3+/ Eu2+ luminescence, good proportionality and good energy resolution. They also have small band-gap leading to higher light yields. Ce3+and Eu2+ are efficient, and the emission wavelengths in the 350-500 nm region matches well with PMTs and a new generation of Siphotodiodes. In this

  1. Assessment of scintillation proxy maps for a scintillation study during geomagnetically quiet and disturbed conditions over Uganda

    NASA Astrophysics Data System (ADS)

    Amabayo, Emirant B.; Jurua, Edward; Cilliers, Pierre J.

    2017-02-01

    The objective of this paper is demonstrate the validity and usefulness of scintillation proxies derived from IGS data, through its comparison with data from dedicated scintillation monitors and its application to GNSS scintillation patterns. The paper presents scintillation patterns developed by using data from the dedicated scintillation monitors of the scintillation network decision aid (SCINDA) network, and proxy maps derived from IGS GPS data for 2011 and 2012 over low latitude stations in Uganda. The amplitude and phase scintillation indicies (S4 and σΦ) were obtained from the Novatel GSV4004B ionospheric scintillation and total electron content (TEC) monitor managed by SCINDA at Makerere (0.340N, 32.570E). The corresponding IGS GPS proxy data were obtained from the receivers at Entebbe (0.040N, 32.440E) and Mbarara (0.600S, 30.740E). The derived amplitude (S4p) and phase (sDPR) scintillation proxy maps were compared with maps of S4 and σΦ during geomagnetic storms (moderate and strong) and geomagnetically quiet conditions. The scintillation patterns using S4 and σΦ and their respective proxies revealed similar diurnal and seasonal patterns of strong scintillation occurrence. The peaks of scintillation occurrence with mean values in the range 0.3 < (S4p , sDPR) ≤ 0.6 were observed during nighttime (17:00-22:00 UT) and in the months of March-April and September-October. The results also indicate that high level scintillations occur during geomagnetically disturbed (moderate and strong) and quiet conditions over the Ugandan region. The results show that SCINDA and IGS based scintillation patterns reveal the same nighttime and seasonal occurrence of irregularities over Uganda irrespective of the geomagnetic conditions. Therefore, the amplitude and phase scintillation proxies presented here can be used to fill gaps in low-latitude data where there are no data available from dedicated scintillation receivers, irrespective of the geomagnetic conditions.

  2. Development of new Polysiloxane Based Liquid Scintillators

    SciTech Connect

    Dalla Palma, M.; Quaranta, A.; Gramegna, F.; Marchi, T.; Cinausero, M.; Carturan, S.; Collazuol, G.; Checchia, C.; Degerlier, M.

    2015-07-01

    In the last decade, attention toward neutron detection has been growing in the scientific community, driven by new requirements in different fields of application ranging from homeland security to medical and material analysis, from research physics, to nuclear energy production. So far neutron detection, with particular attention to fast neutrons, has been mainly based on organic liquid scintillators, owing to their good efficiency and pulse shape discrimination (PSD) capability. Most of these liquids have however some main drawbacks given by toxicity, flammability, volatility and sensitivity to dissolved oxygen that limits the duration and the quality of their performances with worse handiness and increased costs. Phenyl-substituted polysiloxanes could address most of these issues, being characterized by low toxicity, low volatility and low flammability. Their optical properties can be tailored by changing the phenyl distribution and concentration thus allowing to increase the solubility of organic dyes, to modify the fluorescence spectra and to vary the refractive index of the medium. Furthermore, polysiloxanes have been recently exploited for the production of plastic scintillators with very good chemical and thermal stability and very good radiation hardness and the development of polysiloxane liquid scintillators could allow to combine these interesting properties with the supremacy of liquid scintillators as regarding PSD over plastics. For these reasons, the properties of several phenyl-substituted polysiloxane with different phenyl amounts and different viscosities have been investigated, with particular attention to the scintillation response and the pulse shape discrimination capability, and the results of the investigation are reported in this work. More in details, the scintillation light yield towards gamma rays ({sup 60}Co and {sup 137}Cs) of several polysiloxane liquids has been analyzed and compared with the light yield of a commercial non

  3. Robust GPS carrier tracking under ionospheric scintillation

    NASA Astrophysics Data System (ADS)

    Susi, M.; Andreotti, M.; Aquino, M. H.; Dodson, A.

    2013-12-01

    Small scale irregularities present in the ionosphere can induce fast and unpredictable fluctuations of Radio Frequency (RF) signal phase and amplitude. This phenomenon, known as scintillation, can degrade the performance of a GPS receiver leading to cycle slips, increasing the tracking error and also producing a complete loss of lock. In the most severe scenarios, if the tracking of multiple satellites links is prevented, outages in the GPS service can also occur. In order to render a GPS receiver more robust under scintillation, particular attention should be dedicated to the design of the carrier tracking stage, that is the receiver's part most sensitive to these types of phenomenon. This paper exploits the reconfigurability and flexibility of a GPS software receiver to develop a tracking algorithm that is more robust under ionospheric scintillation. For this purpose, first of all, the scintillation level is monitored in real time. Indeed the carrier phase and the post correlation terms obtained by the PLL (Phase Locked Loop) are used to estimate phi60 and S4 [1], the scintillation indices traditionally used to quantify the level of phase and amplitude scintillations, as well as p and T, the spectral parameters of the fluctuations PSD. The effectiveness of the scintillation parameter computation is confirmed by comparing the values obtained by the software receiver and the ones provided by a commercial scintillation monitoring, i.e. the Septentrio PolarxS receiver [2]. Then the above scintillation parameters and the signal carrier to noise density are exploited to tune the carrier tracking algorithm. In case of very weak signals the FLL (Frequency Locked Loop) scheme is selected in order to maintain the signal lock. Otherwise an adaptive bandwidth Phase Locked Loop (PLL) scheme is adopted. The optimum bandwidth for the specific scintillation scenario is evaluated in real time by exploiting the Conker formula [1] for the tracking jitter estimation. The performance

  4. Scintillating fiber detector performance, detector geometries, trigger, and electronics issues for scintillating fiber tracking

    SciTech Connect

    Baumbaugh, A.E.

    1994-06-01

    Scintillating Fiber tracking technology has made great advances and has demonstrated great potential for high speed charged particle tracking and triggering. The small detector sizes and fast scintillation fluors available make them very promising for use at high luminosity experiments at today`s and tomorrow`s colliding and fixed target experiments where high rate capability is essential. This talk will discuss the current state of Scintillating fiber performance and current Visual Light Photon Counter (VLPC) characteristics. The primary topic will be some of the system design and integration issues which should be considered by anyone attempting to design a scintillating fiber tracking system which includes a high speed tracking trigger. Design. constraints placed upon the detector system by the electronics and mechanical sub-systems will be discussed. Seemingly simple and unrelated decisions can have far reaching effects on overall system performance. SDC and DO example system designs will be discussed.

  5. The SNO+ Scintillator Purification Plant and Projected Sensitivity to Solar Neutrinos in the Pure Scintillator Phase

    NASA Astrophysics Data System (ADS)

    Pershing, Teal; SNO+ Collaboration

    2016-03-01

    The SNO+ detector is a neutrino and neutrinoless double-beta decay experiment utilizing the renovated SNO detector. In the second phase of operation, the SNO+ detector will contain 780 tons of organic liquid scintillator composed of 2 g/L 2,5-diphenyloxazole (PPO) in linear alkylbenzene (LAB). In this phase, SNO+ will strive to detect solar neutrinos in the sub-MeV range, including CNO production neutrinos and pp production neutrinos. To achieve the necessary detector sensitivity, a four-part scintillator purification plant has been constructed in SNOLAB for the removal of ionic and radioactive impurities. We present an overview of the SNO+ scintillator purification plant stages, including distillation, water extraction, gas stripping, and metal scavenger columns. We also give the projected SNO+ sensitivities to various solar-produced neutrinos based on the scintillator plant's projected purification efficiency.

  6. Characterizing Scintillation and Cherenkov Light in Water-Based Liquid Scintillators

    NASA Astrophysics Data System (ADS)

    Land, Benjamin; Caravaca, Javier; Descamps, Freija; Orebi Gann, Gabriel

    2016-09-01

    The recent development of Water-based Liquid Scintillator (WbLS) has made it possible to produce scintillating materials with highly tunable light yields and excellent optical clarity. This allows for a straightforward combination of the directional properties of Cherenkov light with the greater energy resolution afforded by the typically brighter scintillation light which lends itself well to a broad program of neutrino physics. Here we explore the light yields and time profiles of WbLS materials in development for Theia (formerly ASDC) as measured in CheSS: our bench-top Cherenkov and scintillation separation R&D project at Berkeley Lab. This work was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231.

  7. Development of scintillator plates with high energy resolution for alpha particles made of GPS scintillator grains

    NASA Astrophysics Data System (ADS)

    Shimaoka, Takehiro; Kaneko, Junichi H.; Izaki, Kenji; Tsubota, Youichi; Higuchi, Mikio; Nishiyama, Shusuke

    2014-01-01

    A scintillator plate with high energy resolution was developed to produce an alpha particle monitor used in nuclear fuel reprocessing plants and mixed plutonium-uranium oxide (MOX) fuel plants. Grains of a Gd2Si2O7 (GPS) scintillator of several 10 to 550 μm were fixed on a glass substrate and were then mechanically polished. By increasing the size of scintillator grains and removing fine powders, the collected light yield and energy resolution for alpha particles were drastically improved. Energy resolution of 9.3% was achieved using average grain size of 91 μm. Furthermore, the ratios between counts in a peak and total counts were improved by more than 60% by the further increase of grain size and adoption of mechanically polished surfaces on both sides. Beta and gamma ray influences were suppressed sufficiently by the thin 100 μm scintillator plates.

  8. Double {beta} experiments with the help of scintillation and HPGe detectors at Gran Sasso

    SciTech Connect

    Barabash, A.; Konovalov, S. I.; Umatov, V. I.; Belli, P.; D'Angelo, S.; Di Marco, A.; Bernabei, R.; Boiko, R. S.; Chernyak, D. M.; Danevich, F. A.; Kobychev, V. V.; Kropivyansky, B. N.; Kudovbenko, V. M.; Nagorny, S. S.; Podviyanuk, R. B.; Polischuk, O. G.; Tretyak, V. I.; Vyshnevskyi, I. M.; Yurchenko, S. S.; Brudanin, V. B.; and others

    2011-12-16

    A search for double beta decay of {sup 64,70}Zn, {sup 180,186}W was carried out by using low background ZnWO{sub 4} crystal scintillators, while a CeCl{sub 3} scintillation detector was applied to investigate 2{beta} processes in {sup 136,138,142}Ce. A search for 2{beta} decay of {sup 96,104}Ru, {sup 156,158}Dy, {sup 190,198}Pt and study of 2{nu}2{beta} decay of {sup 100}Mo to the first excited 0{sup +} level of {sup 100}Ru were realized by ultra-low background HPGe {gamma} spectrometry. Moreover, CdWO{sub 4} crystal scintillators from enriched {sup 106}Cd and {sup 116}Cd isotopes were developed to search for 2{beta} decay of {sup 106}Cd and {sup 116}Cd. Finally, experiments aimed to investigate {sup 96,104}Ru and {sup 116}Cd are in progress and a new phase of the experiment to search for 2{beta} processes in {sup 106}Cd is in preparation.

  9. Liquid Scintillator Production for the NOvA Experiment

    DOE PAGES

    Mufson, S.; Baugh, B.; Bower, C.; ...

    2015-04-15

    The NOvA collaboration blended and delivered 8.8 kt (2.72M gal) of liquid scintillator as the active detector medium to its near and far detectors. The composition of this scintillator was specifically developed to satisfy NOvA's performance requirements. A rigorous set of quality control procedures was put in place to verify that the incoming components and the blended scintillator met these requirements. The scintillator was blended commercially in Hammond, IN. The scintillator was shipped to the NOvA detectors using dedicated stainless steel tanker trailers cleaned to food grade.

  10. Liquid scintillator production for the NOvA experiment

    NASA Astrophysics Data System (ADS)

    Mufson, S.; Baugh, B.; Bower, C.; Coan, T. E.; Cooper, J.; Corwin, L.; Karty, J. A.; Mason, P.; Messier, M. D.; Pla-Dalmau, A.; Proudfoot, M.

    2015-11-01

    The NOvA collaboration blended and delivered 8.8 kt (2.72M gal) of liquid scintillator as the active detector medium to its near and far detectors. The composition of this scintillator was specifically developed to satisfy NOvA's performance requirements. A rigorous set of quality control procedures was put in place to verify that the incoming components and the blended scintillator met these requirements. The scintillator was blended commercially in Hammond, IN. The scintillator was shipped to the NOvA detectors using dedicated stainless steel tanker trailers cleaned to food grade.

  11. Light propagation and fluorescence quantum yields in liquid scintillators

    NASA Astrophysics Data System (ADS)

    Buck, C.; Gramlich, B.; Wagner, S.

    2015-09-01

    For the simulation of the scintillation and Cherenkov light propagation in large liquid scintillator detectors a detailed knowledge about the absorption and emission spectra of the scintillator molecules is mandatory. Furthermore reemission probabilities and quantum yields of the scintillator components influence the light propagation inside the liquid. Absorption and emission properties are presented for liquid scintillators using 2,5-Diphenyloxazole (PPO) and 4-bis-(2-Methylstyryl)benzene (bis-MSB) as primary and secondary wavelength shifter. New measurements of the quantum yields for various aromatic molecules are shown.

  12. Fluorescent compounds for plastic scintillation applications

    SciTech Connect

    Pla-Dalmau, A.; Bross, A.D.

    1994-04-01

    Several 2-(2{prime}-hydroxyphenyl)benzothiazole, -benzoxazole, and -benzimidazole derivatives have been prepared. Transmittance, fluorescence, light yield, and decay time characteristics of these compounds have been studied in a polystyrene matrix and evaluated for use in plastic scintillation detectors. Radiation damage studies utilizing a {sup 60}C source have also been performed.

  13. Scintillator Development for the PROSPECT Experiment

    NASA Astrophysics Data System (ADS)

    Yeh, Minfang

    2014-03-01

    Doped scintillator is the target material of choice for antineutrino detection as it utilizes the time-delayed coincidence signature of the positron annihilation and neutron capture resulting from the Inverse Beta Decay (IBD) interaction. Additionally, the multiple gamma rays or heavy ions emitted after neutron capture on either Gd or 6Li respectively provide a distinct signal for the identification of antineutrino events and therefore significantly enhance accidental background reduction. The choice of scintillator and dopant depends on the detector requirements and scintillator performance criteria. Both Gd and 6Li doped scintillators have been used in past reactor antineutrino experiments such as Double Chooz, Daya Bay, RENO, and Bugey3 and are currently under investigation by the PROSPECT collaboration. Their properties in terms of light yield, optical transparency, chemical stability and background rejection efficiency using Pulse Shape Discrimination (PSD) will be reported. Research sponsored by the U.S. Department of Energy, Office of Nuclear Physics and Office of High Energy Physics, under contract with Brookhaven National Laboratory-Brookhaven Science Associates.

  14. Progress in studying scintillator proportionality: Phenomenological model

    SciTech Connect

    Bizarri, Gregory; Cherepy, Nerine; Choong, Woon-Seng; Hull, Giulia; Moses, William; Payne, Sephen; Singh, Jai; Valentine, John; Vasilev, Andrey; Williams, Richard

    2009-04-30

    We present a model to describe the origin of non-proportional dependence of scintillator light yield on the energy of an ionizing particle. The non-proportionality is discussed in terms of energy relaxation channels and their linear and non-linear dependences on the deposited energy. In this approach, the scintillation response is described as a function of the deposited energy deposition and the kinetic rates of each relaxation channel. This mathematical framework allows both a qualitative interpretation and a quantitative fitting representation of scintillation non-proportionality response as function of kinetic rates. This method was successfully applied to thallium doped sodium iodide measured with SLYNCI, a new facility using the Compton coincidence technique. Finally, attention is given to the physical meaning of the dominant relaxation channels, and to the potential causes responsible for the scintillation non-proportionality. We find that thallium doped sodium iodide behaves as if non-proportionality is due to competition between radiative recombinations and non-radiative Auger processes.

  15. Optimization of Shielded Scintillator for Neutron Detection

    NASA Astrophysics Data System (ADS)

    Belancourt, Patrick; Morrison, John; Akli, Kramer; Freeman, Richard; High Energy Density Physics Team

    2011-10-01

    The High Energy Density Physics group is interested in the basic science of creating a neutron and gamma ray source. The neutrons and gamma rays are produced by accelerating ions via a laser into a target and creating fusion neutrons and gamma rays. A scintillator and photomultiplier tube will be used to detect these neutrons. Neutrons and photons produce ionizing radiation in the scintillator which then activates metastable states. These metastable states have both short and long decay rates. The initial photon count is orders of magnitude higher than the neutron count and poses problems for accurately detecting the neutrons due to the long decay state that is activated by the photons. The effects of adding lead shielding on the temporal response and signal level of the neutron detector will be studied in an effort to minimize the photon count without significant reduction to the temporal resolution of the detector. MCNP5 will be used to find the temporal response and energy deposition into the scintillator by adding lead shielding. Results from the simulations will be shown. Optimization of our scintillator neutron detection system is needed to resolve the neutron energies and neutron count of a novel neutron and gamma ray source.

  16. Equitorial Scintillations: Advances Since ISEA-6.

    DTIC Science & Technology

    1985-01-01

    thermospheric neutral wind have been postulated to describe the observe l longitudinal variation._--.-, A distinct class of equatorial irregularities...Unclassified SECURITY CLASSIFICATION OF THIS PAGE associated with frequency spread on ionograms . Scintillations caused by such irregularities exist only...another based on the influence of a transequatorial thermospheric neutral wind have been postu- lated to describe the observed longitudinal variation. A

  17. Outward atmospheric scintillation effects and inward atmospheric scintillation effects comparisons for direct detection ladar applications

    NASA Astrophysics Data System (ADS)

    Youmans, Douglas G.

    2014-06-01

    Atmospheric turbulence produces intensity modulation or "scintillation" effects on both on the outward laser-mode path and on the return backscattered radiation path. These both degrade laser radar (ladar) target acquisition, ranging, imaging, and feature estimation. However, the finite sized objects create scintillation averaging on the outgoing path and the finite sized telescope apertures produce scintillation averaging on the return path. We expand on previous papers going to moderate to strong turbulence cases by starting from a 20kft altitude platform and propagating at 0° elevation (with respect to the local vertical) for 100km range to a 1 m diameter diffuse sphere. The outward scintillation and inward scintillation effects, as measured at the focal plane detector array of the receiving aperture, will be compared. To eliminate hard-body surface speckle effects in order to study scintillation, Goodman's M-parameter is set to 106 in the analytical equations and the non-coherent imaging algorithm is employed in Monte Carlo realizations. The analytical equations of the signal-to-noise ratio (SNRp), or mean squared signal over a variance, for a given focal plane array pixel window of interest will be summarized and compared to Monte Carlo realizations of a 1m diffuse sphere.

  18. Systematic study of particle quenching in organic scintillators

    NASA Astrophysics Data System (ADS)

    Santiago, L. M.; Bagán, H.; Tarancón, A.; Rauret, G.; Garcia, J. F.

    2013-01-01

    Among the different factors that affect measurements by organic scintillators, the majority of attention has been focused on those related to the scintillator (i.e., ionization, chemical, color and optical quenching), and less attention has been paid to the loss of energy before the particle (i.e., alpha or beta) arrives at the scintillator (i.e., particle quenching). This study evaluates the effect of particle quenching in different scintillation methods (i.e., using two plastic scintillation microspheres (PSm1 and PSm2), liquid scintillator and gel scintillator) by measuring solutions that contain increasing concentrations of NaCl, BaCl2 and glycerin. The results show the importance of particle quenching in PSm measurements because detection efficiency decreases with increasing concentrations of the quenching component, although the spectrum position and external standard parameter remain constant. The results have shown evidence of particle quenching, although at a lower magnitude, in the liquid scintillation or gel scintillation measurements. Moreover, the use of two PSm with different diameters and salty compound that alters the equilibrium of the liquid and gel emulsions also exemplified the importance of the transmission of optical photons through different scintillation media (i.e., optical quenching). Improvement and deterioration of the optical conditions on the scintillation media is manifested as a movement of the spectrum to higher and lower energies, respectively. The results obtained with PSm were confirmed by Monte Carlo simulation.

  19. Synthesis and characterization of a BaGdF5:Tb glass ceramic as a nanocomposite scintillator for x-ray imaging.

    PubMed

    Lee, Gyuhyon; Struebing, Christian; Wagner, Brent; Summers, Christopher; Ding, Yong; Bryant, Alex; Thadhani, Naresh; Shedlock, Daniel; Star-Lack, Josh; Kang, Zhitao

    2016-05-20

    Transparent glass ceramics with embedded light-emitting nanocrystals show great potential as low-cost nanocomposite scintillators in comparison to single crystal and transparent ceramic scintillators. In this study, cubic structure BaGdF5:Tb nanocrystals embedded in an aluminosilicate glass matrix are reported for potential high performance MeV imaging applications. Scintillator samples with systematically varied compositions were prepared by a simple conventional melt-quenching method followed by annealing. Optical, structural and scintillation properties were characterized to guide the design and optimization of selected material systems, aiming at the development of a system with higher crystal volume and larger crystal size for improved luminosity. It is observed that enhanced scintillation performance was achieved by tuning the glass matrix composition and using GdF3 in the raw materials, which served as a nucleation agent. A 26% improvement in light output was observed from a BaGdF5:Tb glass ceramic with addition of GdF3.

  20. Optimizing timing performance of silicon photomultiplier-based scintillation detectors

    PubMed Central

    Yeom, Jung Yeol; Vinke, Ruud

    2013-01-01

    Precise timing resolution is crucial for applications requiring photon time-of-flight (ToF) information such as ToF positron emission tomography (PET). Silicon photomultipliers (SiPM) for PET, with their high output capacitance, are known to require custom preamplifiers to optimize timing performance. In this paper, we describe simple alternative front-end electronics based on a commercial low-noise RF preamplifier and methods that have been implemented to achieve excellent timing resolution. Two radiation detectors with L(Y)SO scintillators coupled to Hamamatsu SiPMs (MPPC S10362–33-050C) and front-end electronics based on an RF amplifier (MAR-3SM+), typically used for wireless applications that require minimal additional circuitry, have been fabricated. These detectors were used to detect annihilation photons from a Ge-68 source and the output signals were subsequently digitized by a high speed oscilloscope for offline processing. A coincident resolving time (CRT) of 147 ± 3 ps FWHM and 186 ± 3 ps FWHM with 3 × 3 × 5 mm3 and with 3 × 3 × 20 mm3 LYSO crystal elements were measured, respectively. With smaller 2 × 2 × 3 mm3 LSO crystals, a CRT of 125 ± 2 ps FWHM was achieved with slight improvement to 121 ± 3 ps at a lower temperature (15°C). Finally, with the 20 mm length crystals, a degradation of timing resolution was observed for annihilation photon interactions that occur close to the photosensor compared to shallow depth-of-interaction (DOI). We conclude that commercial RF amplifiers optimized for noise, besides their ease of use, can produce excellent timing resolution comparable to best reported values acquired with custom readout electronics. On the other hand, as timing performance degrades with increasing photon DOI, a head-on detector configuration will produce better CRT than a side-irradiated setup for longer crystals. PMID:23369872

  1. Structural and optical characterization and scintillator application of hydrothermal-grown ZnO microrods

    NASA Astrophysics Data System (ADS)

    Empizo, Melvin John F.; Santos-Putungan, Alexandra B.; Yamanoi, Kohei; Salazar, Hernanie T.; Anguluan, Eloise P.; Mori, Kazuyuki; Arita, Ren; Minami, Yuki; Luong, Mui Viet; Shimizu, Toshihiko; Estacio, Elmer S.; Somintac, Armando S.; Salvador, Arnel A.; Sarmago, Roland V.; Fukuda, Tsuguo; Sarukura, Nobuhiko

    2017-03-01

    ZnO microrods are fabricated by a simple hydrothermal growth route using zinc acetate dihydrate [Zn(CH3COO)2·2H2O] and hexamethylenetetramine [(CH2)6N4] aqueous solutions. The as-prepared microrods exhibit uniform dimensions, well-faceted surfaces, and hexagonal crystal structure. The microrods also have an intense ultraviolet (UV) emission at 392 nm with an average lifetime of 80 ps. No peaks are observed at the visible wavelengths that can be attributed to defect-related emissions. With excellent structural and optical properties and with loose adhesion to their substrates, the ZnO microrods can be isolated, harvested, and manipulated and can be integrated as building blocks of a microstructured scintillator screen. The proposed scintillator screen possibly offers efficient and precise detection with high resolution. Hydrothermal-grown ZnO microrods then hold a promise towards radiation detector innovation and integrated optoelectronic microsystems.

  2. High-throughput combinatorial database of electronic band structures for inorganic scintillator materials.

    PubMed

    Setyawan, Wahyu; Gaume, Romain M; Lam, Stephanie; Feigelson, Robert S; Curtarolo, Stefano

    2011-07-11

    For the purpose of creating a database of electronic structures of all the known inorganic compounds, we have developed a computational framework based on high-throughput ab initio calculations (AFLOW) and an online repository (www.aflowlib.org). In this article, we report the first step of this task: the calculation of band structures for 7439 compounds intended for the research of scintillator materials for γ-ray radiation detection. Data-mining is performed to select the candidates from 193,456 compounds compiled in the Inorganic Crystal Structure Database. Light yield and scintillation nonproportionality are predicted based on semiempirical band gaps and effective masses. We present a list of materials, potentially bright and proportional, and focus on those exhibiting small effective masses and effective mass ratios.

  3. Development of the Fast Scintillation Detector with Programmable High Voltage Adjustment Suitable for Moessbauer Spectroscopy

    SciTech Connect

    Prochazka, R.; Frydrych, J.; Pechousek, J.

    2010-07-13

    This work is focused on a development of a compact fast scintillation detector suitable for Moessbauer spectroscopy (low energy X-ray/{gamma}-ray detection) where high counting rates are inevitable. Optimization of this part was necessary for a reliable function, better time resolution and to avoid a detector pulses pile-up effect. The pile-up effect decreases the measurement performance, significantly depends on the source activity and also on the pulse duration. Our new detection unit includes a fast scintillation crystal YAP:Ce, an R6095 photomultiplier tube, a high voltage power supply socket C9028-01 assembly, an AD5252 digital potentiometer with an I2C interface and an AD8000 ultra fast operation preamplifier. The main advantages of this solution lie in a short pulse duration (less than 200 ns), stable operation for high activities, programmable gain of the high voltage supply and compact design in the aluminum housing.

  4. C7LYC Scintillators and Fast Neutron Spectroscopy

    NASA Astrophysics Data System (ADS)

    Chowdhury, P.; Brown, T.; Doucet, E.; Lister, C. J.; Wilson, G. L.; D'Olympia, N.; Devlin, M.; Mosby, S.

    2016-09-01

    Cs2 LiYCl6 (CLYC) scintillators detect both gammas and neutrons with excellent pulse shape discrimination. At UML, fast neutron measurements with a 16-element 1''x1'' CLYC array show promise for low energy nuclear science. CLYC detects fast neutrons via the 35Cl (n,p) reaction (resolution < 10 % at < 8 MeV). In our 7Li-enriched C7LYC, the thermal neutron response from the 6Li(n, α)t reaction is virtually eliminated. The low intrinsic efficiency of CLYC for fast neutrons (< 1 %) is offset by increased solid angle with the array placed near the target, since TOF is not needed for energy resolution. The array was tested at LANL for measuring elastic and inelastic neutron scattering on 56Fe. The incident energy from the white neutron source was measured via TOF, and the scattered neutron energy via the pulse height in CLYC. The array was also tested at CARIBU for measuring beta-delayed neutrons. Larger CLYC crystals are now a reality. Measurements with the first 3'' x 3'' C7LYC crystal are in progress at UML. Results will be discussed in the context of constructing a C7LYC array at FRIB for reaction and decay spectroscopy of neutron-rich fragments. Supported by the NNSA Stewardship Science Academic Alliance Program under Grant DE-NA00013008.

  5. Processing of transparent polycrystalline AlON:Ce3+ scintillators

    DOE PAGES

    Chen, Ching -Fong; Yang, Pin; King, Graham; ...

    2015-10-23

    A new polycrystalline ceramic scintillator is reported for potential use in radiation detection and medical imaging applications. The goal was to develop cerium-activated aluminum oxynitride (AlON:Ce3+) ceramics, which can be produced using ceramic processes in comparison to the high-cost, low-yield single-crystal growth technique. A phase pure AlON:Ce3+ powder with cubic symmetry was successfully synthesized at high temperature under a reducing atmosphere to convert Ce4+ to Ce3+ in the solid solution. We explored two different activator concentrations (0.5 and 1.0 mol%). Fully dense and transparent AlON:Ce3+ ceramics were produced by a liquid-phase-assisted pressureless sintering. The crystal field splitting around the Ce3+more » activator in the AlON was comparable to the splitting induced by Br₋ and the Cl₋ ligands, which produced an emission spectrum perfectly matching the maximum quantum efficiency range of the photomultiplier tube for radiation detection. Both optical excitation and radiation ionizations in AlON:Ce3+ were demonstrated. Lastly, challenges and mechanisms related to the radioluminescence efficiency are discussed.« less

  6. LuAlO{sub 3}: A high density, high speed scintillator for gamma detection

    SciTech Connect

    Moses, W.W.; Derenzo, S.E.; Fyodorov, A.; Korzhik, M.; Gektin, A.; Minkov, B.; Aslanov, V.

    1994-11-01

    We present measurements of the scintillation properties cerium doped lutetium aluminum perovskite, LuAlO{sub 3}:C, new dense ({rho}=8.34 g/cm{sup 3}) inorganic scintillator. This material has a 511 keV interaction length and photoelectric fraction 1.1 cm and 32% respectively, which are well suited to gamma ray detection. In powdered form with 0.5% cerium concentration, the scintillation light output is estimated to be 9,600 photons/MeV of deposited energy, the emission spectrum is a single peak centered at 390 nm, and the fluorescence lifetime is described by the sum of 3 exponential terms, with 60% of the light being emitted with a 11 ns decay time, 26% with a 28 ns decay time, and 13% with a 835 ns decay time. Single crystals contaminated with =10% lutetium aluminum garnet (Lu{sub 3}Al{sub 5}O{sub l2}) have significantly altered scintillation properties. The light output is 26,000 photons/MeV (3.2 times that of BGO), but the decay time increases significantly (1% of the light is emitted with a 10 ns decay time, 15% with a 245 ns decay time, and 85% with a 2010 ns decay time) and the emission spectrum is dominated by a peak centered at 315 nm with a secondary peak centered at 500 rum. The short decay lifetime, high density, and reasonable light output of LuAlO{sub 3}:C (the perovskite phase) suggest that it is useful for applications where high counting rates, good stopping power, good energy resolution, and fast timing are important. However, it is necessary to grow single crystals that are uncontaminated by the garnet phase to realize these properties.

  7. Thermal neutron detection using alkali halide scintillators with Li-6 and pulse shape discrimination

    SciTech Connect

    Brubaker, Erik; Dibble, Dean C.; Mengesha, Wondwosen; Yang, Pin

    2013-09-01

    An ideal 3He detector replacement for the near- to medium-term future will use materials that are easy to produce and well understood, while maintaining thermal neutron detection efficiency and gamma rejection close to the 3He standard. Toward this end, we investigated the use of standard alkali halide scintillators interfaced with 6Li and read out with photomultiplier tubes (PMTs). Thermal neutrons are captured on 6Li with high efficiency, emitting high-energy and triton (3H) reaction products. These particles deposit energy in the scintillator, providing a thermal neutron signal; discrimination against gamma interactions is possible via pulse shape discrimination (PSD), since heavy particles produce faster pulses in alkali halide crystals. We constructed and tested two classes of detectors based on this concept. In one case 6Li is used as a dopant in polycrystalline NaI; in the other case a thin Li foil is used as a conversion layer. In the configurations studied here, these systems are sensitive to both gamma and neutron radiation, with discrimination between the two and good energy resolution for gamma spectroscopy. We present results from our investigations, including measurements of the neutron efficiency and gamma rejection for the two detector types. We also show a comparison with Cs2LiYCl6:Ce (CLYC), which is emerging as the standard scintillator for simultaneous gamma and thermal neutron detection, and also allows PSD. We conclude that 6Li foil with CsI scintillating crystals has near-term promise as a thermal neutron detector in applications previously dominated by 3He detectors. The other approach, 6Li-doped alkali halides, has some potential, but require more work to understand material properties and improve fabrication processes.

  8. Relative light yield and temporal response of a stilbene-doped bibenzyl organic scintillator for neutron detection

    SciTech Connect

    Brown, J. A.; Goldblum, B. L. Brickner, N. M.; Daub, B. H.; Kaufman, G. S.; Bibber, K. van; Vujic, J.; Bernstein, L. A.; Bleuel, D. L.; Caggiano, J. A.; Hatarik, R.; Phillips, T. W.; Zaitseva, N. P.; Wender, S. A.

    2014-05-21

    The neutron time-of-flight (nTOF) diagnostics used to characterize implosions at the National Ignition Facility (NIF) has necessitated the development of novel scintillators that exhibit a rapid temporal response and high light yield. One such material, a bibenzyl-stilbene mixed single-crystal organic scintillator grown in a 99.5:0.5 ratio in solution, has become the standard scintillator used for nTOF diagnostics at NIF. The prompt fluorescence lifetime and relative light yield as a function of proton energy were determined to calibrate this material as a neutron detector. The temporal evolution of the intensity of the prompt fluorescent response was modeled using first-order reaction kinetics and the prompt fluorescence decay constant was determined to be 2.46 ± 0.01 (fit) ± 0.13 (systematic) ns. The relative response of the bibenzyl-stilbene mixed crystal generated by recoiling protons was measured, and results were analyzed using Birks' relation to quantify the non-radiative quenching of excitation energy in the scintillator.

  9. A feasibility study of ortho-positronium decays measurement with the J-PET scanner based on plastic scintillators

    NASA Astrophysics Data System (ADS)

    Kamińska, D.; Gajos, A.; Czerwiński, E.; Alfs, D.; Bednarski, T.; Białas, P.; Curceanu, C.; Dulski, K.; Głowacz, B.; Gupta-Sharma, N.; Gorgol, M.; Hiesmayr, B. C.; Jasińska, B.; Korcyl, G.; Kowalski, P.; Krzemień, W.; Krawczyk, N.; Kubicz, E.; Mohammed, M.; Niedźwiecki, Sz.; Pawlik-Niedźwiecka, M.; Raczyński, L.; Rudy, Z.; Silarski, M.; Wieczorek, A.; Wiślicki, W.; Zgardzińska, B.; Zieliński, M.; Moskal, P.

    2016-08-01

    We present a study of the application of the Jagiellonian positron emission tomograph (J-PET) for the registration of gamma quanta from decays of ortho-positronium (o-Ps). The J-PET is the first positron emission tomography scanner based on organic scintillators in contrast to all current PET scanners based on inorganic crystals. Monte Carlo simulations show that the J-PET as an axially symmetric and high acceptance scanner can be used as a multi-purpose detector well suited to pursue research including e.g. tests of discrete symmetries in decays of ortho-positronium in addition to the medical imaging. The gamma quanta originating from o-Ps decay interact in the plastic scintillators predominantly via the Compton effect, making the direct measurement of their energy impossible. Nevertheless, it is shown in this paper that the J-PET scanner will enable studies of the { o-Ps }→ 3γ decays with angular and energy resolution equal to σ (θ ) ≈ {0.4°} and σ (E) ≈ 4.1 {keV}, respectively. An order of magnitude shorter decay time of signals from plastic scintillators with respect to the inorganic crystals results not only in better timing properties crucial for the reduction of physical and instrumental background, but also suppresses significantly the pile-ups, thus enabling compensation of the lower efficiency of the plastic scintillators by performing measurements with higher positron source activities.

  10. A study on dual readout crystal calorimeter for hadron and jet energy measurement at a future lepton collider

    SciTech Connect

    Yeh, G.P.; /Fermilab

    2010-01-01

    Studies of requirements and specifications of crystals are necessary to develop a new generation of crystals for dual readout crystal hadron or total absorption calorimeter. This is a short and basic study of the characteristics and hadron energy measurement of PbWO4 and BGO crystals for scintillation and Cerenkov Dual Readout hadron calorimeter.

  11. Real-time Scintillation Monitoring in Alaska from a Longitudinal Chain of ASTRA's SM-211 GPS TEC and Scintillation Receivers

    NASA Astrophysics Data System (ADS)

    Crowley, G.; Azeem, S. I.; Reynolds, A.; Santana, J.; Hampton, D. L.

    2013-12-01

    Amplitude and phase scintillation can cause serious difficulties for GPS receivers. Intense scintillation can cause loss of lock. High latitude studies generally show that phase scintillation can be severe, but the amplitude scintillation tends to be small. The reason for this is not yet understood. Furthermore, the actual causes of the ionospheric irregularities that produce high latitude scintillation are not well understood. While the gradient drift instability is thought to be important in the F-region, there may be other structures present in either the E- or F-regions. The role of particle precipitation is also not well understood. Four of ASTRA's CASES GPS receivers were deployed in Alaska to demonstrate our ability to map scintillation in realtime, to provide space weather services to GPS users, and to initiate a detailed investigation of these effects. These dual-frequency GPS receivers measure total electron content (TEC) and scintillation. The scintillation monitors were deployed in a longitudinal chain at sites in Kaktovic, Fort Yukon, Poker Flat, and Gakona. Scintillation statistics show phase scintillations to be largest at Kaktovic and smallest at Gakona. We present GPS phase scintillation and auroral emission results from the Alaska chain to characterize the correspondence between scintillation and auroral features, and to investigate the role of high latitude auroral features in driving the phase scintillations. We will also present data showing how phase scintillation can cause other GPS receivers to lose lock. The data and results are particularly valuable because they illustrate some of the challenges of using GPS systems for positioning and navigation in an auroral region like Alaska. These challenges for snowplough drivers were recently highlighted, along with the CASES SM-211 space weather monitor, in a special video in which ASTRA and three other small businesses were presented with an entrepreneurial award from William Shatner (http://youtu.be/bIVKEQH_YPk).

  12. Thallium magnesium chloride: A high light yield, large effective atomic number, intrinsically activated crystalline scintillator for X-ray and gamma-ray detection

    NASA Astrophysics Data System (ADS)

    Fujimoto, Yutaka; Koshimizu, Masanori; Yanagida, Takayuki; Okada, Go; Saeki, Keiichiro; Asai, Keisuke

    2016-09-01

    We report the luminescence and the scintillation properties of a newly developed thallium magnesium chloride (TlMgCl3) crystal. The crystal sample can be easily fabricated from the melt using the Bridgman method. The photoluminescence band appeared near the wavelength of 405 nm under excitation at 230 nm. An X-ray-induced scintillation spectrum showed an intense emission band near the wavelength of 405 nm. The decay time constant was estimated to be approximately 60 ns (∼25%) and 350 ns (∼75%) using a bi-exponential fitting. The scintillation light yield reached 46,000 photons/MeV with an energy resolution of 5% at 662 keV.

  13. Nonproportionality of Scintillator Detectors: Theory and Experiment

    SciTech Connect

    Payne, Stephen; Cherepy, Nerine; Hull, Giulia; Valentine, John; Moses, William; Choong, Woon-Seng

    2009-08-17

    On the basis of nonproportionality data obtained for several scintillators, we have developed a theory to describe the carrier dynamics to fit the light yield versus electron energy. The theory of Onsager was adapted to explain how the carriers form excitons or sequentially arrive at the activators to promote the ion to an excited state, and the theory of Birks was employed to allow for exciton-exciton annihilation. We then developed a second theory to deduce the degradation in resolution that results from nonproportionality by evoking Landau fluctuations, which are essentially variations in the deposited energy density that occur as the high energy electron travels along its trajectory. In general there is good agreement with the data, in terms of fitting the nonproportionality curves and reproducing the literature values of nonproportionality's contribution to the scintillator resolution. With the resurgence of interest in developing scintillator detectors that have good energy resolution, an improved understanding of nonproportionality has become a crucial matter since it presents the fundamental limit to the achievable resolution. In order to hasten an improved understanding of scintillator nonproportionality, we have constructed an instrument referred to as SLYNCI (Scintillator Light Yield Nonproportionality Compton Instrument). This is a second-generation instrument to the original device developed by Valentine and coworkers, wherein several new principles of operation have served to increase the data rate by an order of magnitude as discussed in detail in References. In the present article, the focus is on a theory to describe the measured electron response, which is the light yield as a function of the electron energy. To do this, we account for transport of carriers and excitons, in terms of how they transfer their energy to the activators with competition from nonradiative decay pathways. This work builds on the original work of Murray and coworkers, and

  14. Neutron spectroscopy with scintillation detectors using wavelets

    NASA Astrophysics Data System (ADS)

    Hartman, Jessica

    The purpose of this research was to study neutron spectroscopy using the EJ-299-33A plastic scintillator. This scintillator material provided a novel means of detection for fast neutrons, without the disadvantages of traditional liquid scintillation materials. EJ-299-33A provided a more durable option to these materials, making it less likely to be damaged during handling. Unlike liquid scintillators, this plastic scintillator was manufactured from a non-toxic material, making it safer to use, as well as easier to design detectors. The material was also manufactured with inherent pulse shape discrimination abilities, making it suitable for use in neutron detection. The neutron spectral unfolding technique was developed in two stages. Initial detector response function modeling was carried out through the use of the MCNPX Monte Carlo code. The response functions were developed for a monoenergetic neutron flux. Wavelets were then applied to smooth the response function. The spectral unfolding technique was applied through polynomial fitting and optimization techniques in MATLAB. Verification of the unfolding technique was carried out through the use of experimentally determined response functions. These were measured on the neutron source based on the Van de Graff accelerator at the University of Kentucky. This machine provided a range of monoenergetic neutron beams between 0.1 MeV and 24 MeV, making it possible to measure the set of response functions of the EJ-299-33A plastic scintillator detector to neutrons of specific energies. The response of a plutonium-beryllium (PuBe) source was measured using the source available at the University of Nevada, Las Vegas. The neutron spectrum reconstruction was carried out using the experimentally measured response functions. Experimental data was collected in the list mode of the waveform digitizer. Post processing of this data focused on the pulse shape discrimination analysis of the recorded response functions to remove the

  15. Ce-doped single crystal and ceramic garnets for γ ray detection

    SciTech Connect

    Hull, G; Roberts, J; Kuntz, J; Fisher, S; Sanner, R; Tillotson, T; Drobshoff, A; Payne, S; Cherepy, N

    2007-07-30

    Ceramic and single crystal Lutetium Aluminum Garnet scintillators exhibit energy resolution with bialkali photomultiplier tube detection as good as 8.6% at 662 keV. Ceramic fabrication allows production of garnets that cannot easily be grown as single crystals, such as Gadolinium Aluminum Garnet and Terbium Aluminum Garnet. Measured scintillation light yields of Cerium-doped ceramic garnets indicate prospects for high energy resolution.

  16. Measurement of intrinsic rise times for various L(Y)SO and LuAG scintillators with a general study of prompt photons to achieve 10 ps in TOF-PET.

    PubMed

    Gundacker, Stefan; Auffray, Etiennette; Pauwels, Kristof; Lecoq, Paul

    2016-04-07

    The coincidence time resolution (CTR) of scintillator based detectors commonly used in positron emission tomography is well known to be dependent on the scintillation decay time (τd) and the number of photons detected (n'), i.e. CTR proportional variant √τd/n'. However, it is still an open question to what extent the scintillation rise time (τr) and other fast or prompt photons, e.g. Cherenkov photons, at the beginning of the scintillation process influence the CTR. This paper presents measurements of the scintillation emission rate for different LSO type crystals, i.e. LSO:Ce, LYSO:Ce, LSO:Ce codoped Ca and LGSO:Ce. For the various LSO-type samples measured we find an average value of 70 ps for the scintillation rise time, although some crystals like LSO:Ce codoped Ca seem to have a much faster rise time in the order of 20 ps. Additional measurements for LuAG:Ce and LuAG:Pr show a rise time of 535 ps and 251 ps, respectively. For these crystals, prompt photons (Cherenkov) can be observed at the beginning of the scintillation event. Furthermore a significantly lower rise time value is observed when codoping with calcium. To quantitatively investigate the influence of the rise time to the time resolution we measured the CTR with the same L(Y)SO samples and compared the values to Monte Carlo simulations. Using the measured relative light yields, rise- and decay times of the scintillators we are able to quantitatively understand the measured CTRs in our simulations. Although the rise time is important to fully explain the CTR variation for the different samples tested we determined its influence on the CTR to be in the order of a few percent only. This result is surprising because, if only photonstatistics of the scintillation process is considered, the CTR would be proportional to the square root of the rise time. The unexpected small rise time influence on the CTR can be explained by the convolution of the scintillation rate with the single photon time

  17. Measurement of intrinsic rise times for various L(Y)SO and LuAG scintillators with a general study of prompt photons to achieve 10 ps in TOF-PET

    NASA Astrophysics Data System (ADS)

    Gundacker, Stefan; Auffray, Etiennette; Pauwels, Kristof; Lecoq, Paul

    2016-04-01

    The coincidence time resolution (CTR) of scintillator based detectors commonly used in positron emission tomography is well known to be dependent on the scintillation decay time ({τd} ) and the number of photons detected ({{n}\\prime} ), i.e. CTR\\propto \\sqrt{{τd}/{{n}\\prime}} . However, it is still an open question to what extent the scintillation rise time ({τr} ) and other fast or prompt photons, e.g. Cherenkov photons, at the beginning of the scintillation process influence the CTR. This paper presents measurements of the scintillation emission rate for different LSO type crystals, i.e. LSO:Ce, LYSO:Ce, LSO:Ce codoped Ca and LGSO:Ce. For the various LSO-type samples measured we find an average value of 70 ps for the scintillation rise time, although some crystals like LSO:Ce codoped Ca seem to have a much faster rise time in the order of 20 ps. Additional measurements for LuAG:Ce and LuAG:Pr show a rise time of 535 ps and 251 ps, respectively. For these crystals, prompt photons (Cherenkov) can be observed at the beginning of the scintillation event. Furthermore a significantly lower rise time value is observed when codoping with calcium. To quantitatively investigate the influence of the rise time to the time resolution we measured the CTR with the same L(Y)SO samples and compared the values to Monte Carlo simulations. Using the measured relative light yields, rise- and decay times of the scintillators we are able to quantitatively understand the measured CTRs in our simulations. Although the rise time is important to fully explain the CTR variation for the different samples tested we determined its influence on the CTR to be in the order of a few percent only. This result is surprising because, if only photonstatistics of the scintillation process is considered, the CTR would be proportional to the square root of the rise time. The unexpected small rise time influence on the CTR can be explained by the convolution of the scintillation rate with the

  18. Monitoring and Forecasting Ionospheric Scintillation at High Latitudes (Invited)

    NASA Astrophysics Data System (ADS)

    Prikryl, P.; Jayachandran, P. T.; Chadwick, R.; Kelly, T.

    2013-12-01

    Ionospheric scintillation (rapid signal amplitude fading and phase fluctuation) poses a threat to reliable and safe operation of modern technology that relies on Global Navigation Satellite Systems (GNSS). Ionospheric scintillation of GNSS signal severely degrades positional accuracy, causes cycle slips leading to loss of lock that affects performance of radio communication and navigation systems. At high latitudes, the scintillation is caused by ionospheric irregularities produced through coupling between solar wind plasma and the magnetosphere. Climatology of GPS scintillation at high latitudes in both hemispheres shows that phase scintillation occurs predominantly on the dayside in the cusp and in the nightside auroral oval. Solar wind disturbances, in particular the co-rotating interaction regions (CIR) on the leading edge of high-speed streams (HSS) and interplanetary coronal mass ejections (ICME), have been closely correlated with the occurrence of scintillation at high latitudes. These results demonstrated a technique of probabilistic forecast of high-latitude phase scintillation occurrence relative to arrival times of HSS and ICME. The Canadian High Arctic Ionospheric Network (CHAIN) has been monitoring GPS ionospheric scintillation and total electron content (TEC) since November 2007. One-minute amplitude and phase scintillation indices from L1 GPS signals and TEC from L1 and L2 GPS signals are computed from amplitude and phase data sampled at 50 Hz. Since 2012, significant expansion of CHAIN has begun with installation of new receivers, each capable of tracking up to 30 satellites including GLONASS and Galileo. The receivers log the raw phase and amplitude of the signal up to a 100-Hz rate for scintillation measurements. We briefly review observations of ionospheric scintillation and highlight new results from CHAIN, including the climatology of scintillation occurrence, collocation with aurora and HF radar backscatter, correlation with CIRs and ICMEs

  19. Codoped direct-gap semiconductor scintillators

    DOEpatents

    Derenzo, Stephen E.; Bourret-Courchesne, Edith; Weber, Marvin J.; Klintenberg, Mattias K.

    2006-05-23

    Fast, bright inorganic scintillators at room temperature are based on radiative electron-hole recombination in direct-gap semiconductors, e.g. CdS and ZnO. The direct-gap semiconductor is codoped with two different impurity atoms to convert the semiconductor to a fast, high luminosity scintillator. The codopant scheme is based on dopant band to dopant trap recombination. One dopant provides a significant concentration of carriers of one type (electrons or holes) and the other dopant traps carriers of the other type. Examples include CdS:In,Te; CdS:In,Ag; CdS:In,Na; ZnO:Ga,P; ZnO:Ga,N; ZnO:Ga,S; and GaN:Ge,Mg.

  20. Plastic scintillator detector for pulsed flux measurements

    NASA Astrophysics Data System (ADS)

    Kadilin, V. V.; Kaplun, A. A.; Taraskin, A. A.

    2017-01-01

    A neutron detector, providing charged particle detection capability, has been designed. The main purpose of the detector is to measure pulsed fluxes of both charged particles and neutrons during scientific experiments. The detector consists of commonly used neutron-sensitive ZnS(Ag) / 6LiF scintillator screens wrapping a layer of polystyrene based scintillator (BC-454, EJ-254 or equivalent boron loaded plastic). This type of detector design is able to log a spatial distribution of events and may be scaled to any size. Different variations of the design were considered and modelled in specialized toolkits. The article presents a review of the detector design features as well as simulation results.

  1. Scintillating 99Tc Selective Ion Exchange Resins

    SciTech Connect

    Mitchell Greenhalgh; Richard D. Tillotson

    2012-07-01

    Scintillating technetium (99Tc) selective ion exchange resins have been developed and evaluated for equilibrium capacities and detection efficiencies. These resins can be utilized for the in-situ concentration and detection of low levels of pertechnetate anions (99TcO4-) in natural waters. Three different polystyrene type resin support materials were impregnated with varying amounts of tricaprylmethylammonium chloride (Aliquat 336) extractant, several different scintillating fluors and wavelength shifters. The prepared resins were contacted batch-wise to equilibrium over a wide range of 99TcO4- concentrations in natural water. The measured capacities were used to develop Langmuir adsorption isotherms for each resin. 99Tc detection efficiencies were determined and up to 71.4 ± 2.6% was achieved with some resins. The results demonstrate that a low level detection limit for 99TcO4- in natural waters can be realized.

  2. Reflectance of polytetrafluoroethylene for xenon scintillation light

    SciTech Connect

    Silva, C.; Pinto da Cunha, J.; Pereira, A.; Chepel, V.; Lopes, M. I.; Solovov, V.; Neves, F.

    2010-03-15

    Gaseous and liquid xenon particle detectors are being used in a number of applications including dark matter search and neutrino-less double beta decay experiments. Polytetrafluoroethylene (PTFE) is often used in these detectors both as electrical insulator and as a light reflector to improve the efficiency of detection of scintillation photons. However, xenon emits in the vacuum ultraviolet (VUV) wavelength region ({lambda}{approx_equal}175 nm) where the reflecting properties of PTFE are not sufficiently known. In this work, we report on measurements of PTFE reflectance, including its angular distribution, for the xenon scintillation light. Various samples of PTFE, manufactured by different processes (extruded, expanded, skived, and pressed) have been studied. The data were interpreted with a physical model comprising both specular and diffuse reflections. The reflectance obtained for these samples ranges from about 47% to 66% for VUV light. Other fluoropolymers, namely, ethylene tetrafluoroethylene (ETFE), fluorinated ethylene propylene (FEP), and perfluoro-alkoxyalkane (PFA) were also measured.

  3. Plastic fiber scintillator response to fast neutrons

    SciTech Connect

    Danly, C. R.; Sjue, S.; Wilde, C. H.; Merrill, F. E.; Haight, R. C.

    2014-11-15

    The Neutron Imaging System at NIF uses an array of plastic scintillator fibers in conjunction with a time-gated imaging system to form an image of the neutron emission from the imploded capsule. By gating on neutrons that have scattered from the 14.1 MeV DT energy to lower energy ranges, an image of the dense, cold fuel around the hotspot is also obtained. An unmoderated spallation neutron beamline at the Weapons Neutron Research facility at Los Alamos was used in conjunction with a time-gated imaging system to measure the yield of a scintillating fiber array over several energy bands ranging from 1 to 15 MeV. The results and comparison to simulation are presented.

  4. Codoped direct-gap semiconductor scintillators

    DOEpatents

    Derenzo, Stephen Edward; Bourret-Courchesne, Edith; Weber, Marvin J.; Klintenberg, Mattias K.

    2008-07-29

    Fast, bright inorganic scintillators at room temperature are based on radiative electron-hole recombination in direct-gap semiconductors, e.g. CdS and ZnO. The direct-gap semiconductor is codoped with two different impurity atoms to convert the semiconductor to a fast, high luminosity scintillator. The codopant scheme is based on dopant band to dopant trap recombination. One dopant provides a significant concentration of carriers of one type (electrons or holes) and the other dopant traps carriers of the other type. Examples include CdS:In,Te; CdS:In,Ag; CdS:In,Na; ZnO:Ga,P; ZnO:Ga,N; ZnO:Ga,S; and GaN:Ge,Mg.

  5. Nanophosphor composite scintillators comprising a polymer matrix

    DOEpatents

    Muenchausen, Ross Edward; Mckigney, Edward Allen; Gilbertson, Robert David

    2010-11-16

    An improved nanophosphor composite comprises surface modified nanophosphor particles in a solid matrix. The nanophosphor particle surface is modified with an organic ligand, or by covalently bonding a polymeric or polymeric precursor material. The surface modified nanophosphor particle is essentially charge neutral, thereby preventing agglomeration of the nanophosphor particles during formation of the composite material. The improved nanophosphor composite may be used in any conventional scintillator application, including in a radiation detector.

  6. Sorohalide scintillators, phosphors, and uses thereof

    SciTech Connect

    Yang, Pin; Deng, Haoran; Doty, F. Patrick; Zhou, Xiaowang

    2016-05-10

    The present invention relates to sorohalide compounds having formula A.sub.3B.sub.2X.sub.9, where A is an alkali metal, B is a rare earth metal, and X is a halogen. Optionally, the sorohalide includes a dopant D. Such undoped and doped sorohalides are useful as scintillation materials or phosphors for any number of uses, including for radiation detectors, solid-state light sources, gamma-ray spectroscopy, medical imaging, and drilling applications.

  7. Characteristics of Yerevan High Transparency Scintillators

    SciTech Connect

    Zorn, Carl; Asryan, Gegham; Egiyan, Kim; Tarverdyan, M.; Amaryan, Moscov; Amaryan, Moskov; Demirchyan, Raphael; Stepanyan, Stepan; Burkert, Volker; Sharabian, Youri

    1992-08-01

    Optical transmission, light output and time characteristics are given for long scintillator strips fabricated at the Yerevan Physics Institute using the extrusion method. It is shown that at 45% relative (to anthracene) light output, good transmission (2.5/2.9 m attenuation length with photomultiplier direct readout and 3/3.5 m attenuation length fiber readout) and time characteristics (average decay time 2.8 nsec) were obtained.

  8. Simulating Silicon Photomultiplier Response to Scintillation Light.

    PubMed

    Jha, Abhinav K; van Dam, Herman T; Kupinski, Matthew A; Clarkson, Eric

    2013-02-01

    The response of a Silicon Photomultiplier (SiPM) to optical signals is affected by many factors including photon-detection efficiency, recovery time, gain, optical crosstalk, afterpulsing, dark count, and detector dead time. Many of these parameters vary with overvoltage and temperature. When used to detect scintillation light, there is a complicated non-linear relationship between the incident light and the response of the SiPM. In this paper, we propose a combined discrete-time discrete-event Monte Carlo (MC) model to simulate SiPM response to scintillation light pulses. Our MC model accounts for all relevant aspects of the SiPM response, some of which were not accounted for in the previous models. We also derive and validate analytic expressions for the single-photoelectron response of the SiPM and the voltage drop across the quenching resistance in the SiPM microcell. These analytic expressions consider the effect of all the circuit elements in the SiPM and accurately simulate the time-variation in overvoltage across the microcells of the SiPM. Consequently, our MC model is able to incorporate the variation of the different SiPM parameters with varying overvoltage. The MC model is compared with measurements on SiPM-based scintillation detectors and with some cases for which the response is known a priori. The model is also used to study the variation in SiPM behavior with SiPM-circuit parameter variations and to predict the response of a SiPM-based detector to various scintillators.

  9. a Subminiature Scintillation Detector for Catheter Operation

    NASA Astrophysics Data System (ADS)

    Scafè, R.; Montani, L.; Burgio, N.; Iurlaro, G.; Santagata, A.; Ciavola, C.; Alonge, G.

    2006-04-01

    The feasibility of a subminiature scintillation detector to be inserted in a catheter for lesion localization in nuclear medicine SPECT has been studied. Measurements on a simple laboratory setup have been performed and compared with Monte Carlo results. Further simulations, at 30keV and 140keV, concerning a configuration reproducing severe clinical conditions have shown poor lesion detectability. Several factors affecting the response have to be investigated to improve the capability of lesion localization characterizing such detector.

  10. Improved Neutron Scintillators Based on Nanomaterials

    SciTech Connect

    Dennis Friesel, PhD

    2008-06-30

    The development work conducted in this SBIR has so far not supported the premise that using nano-particles in LiFZnS:Ag foils improves their transparency to 420 (or other frequency) light. This conclusion is based solely on the light absorption properties of LiFZnS foils fabricated from nano- and from micro-particles. Furthermore, even for the case of the Gd{sub 2}O{sub 3} foils, the transmission of 420 nm light gained by using nano-particles all but disappears as the foil thickness is increased beyond about 0.2 mm, a practical scintillator thickness. This was not immediately apparent from the preliminary study since no foils thicker than about 0.04 mm were produced. Initially it was believed that the failure to see an improvement by using nano-particles for the LiFZnS foils was caused by the clumping of the particles in Toluene due to the polarity of the ZnS particles. However, we found, much to our surprise, that nano-particle ZnS alone in polystyrene, and in Epoxy, had worse light transmission properties than the micro-particle foils for equivalent thickness and density foils. The neutron detection measurements, while disappointing, are attributable to our inability to procure or fabricate Bulk Doped ZnS nanoparticles. The cause for the failure of nano-particles to improve the scintillation light, and hence improved neutron detection efficiency, is a fundamental one of light scattering within the scintillator. A consequence of PartTec's documentation of this is that several concepts for the fabrication of improved {sup 6}LiFZnS scintillators were formulated that will be the subject of a future SBIR submission.

  11. Studies of NICADD Extruded Scintillator Strips

    SciTech Connect

    Dychkant, Alexandre; et al.

    2005-03-01

    About four hundred one meter long, 10 cm wide and 5 mm thick extruded scintillating strips were measured at four different points. The results of measurements strip responses to a radioactive source {sup 90}Sr are provided, and details of strip choice, preparation, and method of measurement are included. This work was essential for prototyping a tail catcher and muon tracker for a future international electron positron linear collider detector.

  12. Simulating Scintillator Light Collection Using Measured Optical Reflectance

    SciTech Connect

    Janecek, Martin; Moses, William

    2010-01-28

    To accurately predict the light collection from a scintillating crystal through Monte Carlo simulations, it is crucial to know the angular distribution from the surface reflectance. Current Monte Carlo codes allow the user to set the optical reflectance to a linear combination of backscatter spike, specular spike, specular lobe, and Lambertian reflections. However, not all light distributions can be expressed in this way. In addition, the user seldom has the detailed knowledge about the surfaces that is required for accurate modeling. We have previously measured the angular distributions within BGO crystals and now incorporate these data as look-up-tables (LUTs) into modified Geant4 and GATE Monte Carlo codes. The modified codes allow the user to specify the surface treatment (ground, etched, or polished), the attached reflector (Lumirror(R), Teflon(R), ESR film, Tyvek(R), or TiO paint), and the bonding type (air-coupled or glued). Each LUT consists of measured angular distributions with 4o by 5o resolution in theta and phi, respectively, for incidence angles from 0? to 90? degrees, in 1o-steps. We compared the new codes to the original codes by running simulations with a 3 x 10 x 30 mm3 BGO crystal coupled to a PMT. The simulations were then compared to measurements. Light output was measured by counting the photons detected by the PMT with the 3 x 10, 3 x 30, or 10 x 30 mm2 side coupled to the PMT, respectively. Our new code shows better agreement with the measured data than the current Geant4 code. The new code can also simulate reflector materials that are not pure specular or Lambertian reflectors, as was previously required. Our code is also more user friendly, as no detailed knowledge about the surfaces or light distributions is required from the user.

  13. Boron-Loaded Silicone Rubber Scintillators

    SciTech Connect

    Bell, Z.W.; Maya, L.; Brown, G.M.; Sloop, F.V.Jr

    2003-05-12

    Silicone rubber received attention as an alternative to polyvinyltoluene in applications in which the scintillator is exposed to high doses because of the increased resistance of the rubber to the formation of blue-absorbing color centers. Work by Bowen, et al., and Harmon, et al., demonstrated their properties under gamma/x-ray irradiation, and Bell, et al. have shown their response to thermal neutrons. This last work, however, provided an example of a silicone in which both the boron and the scintillator were contained in the rubber as solutes, a formulation which led to the precipitation of solids and sublimation of the boron component. In the present work we describe a scintillator in which the boron is chemically bonded to the siloxane and so avoids the problem of precipitation and loss of boron to sublimation. Material containing up to 18% boron, by weight, was prepared, mounted on photomultipliers, and exposed to both neutron and gamma fluxes. Pulse height spectra showing the neutron and photon response were obtained, and although the light output was found to be much poorer than from samples in which boron was dissolved, the higher boron concentrations enabled essentially 100% neutron absorption in only a few millimeters' thickness of rubber.

  14. Detecting dark matter with scintillating bubble chambers

    NASA Astrophysics Data System (ADS)

    Zhang, Jianjie; Dahl, C. Eric; Jin, Miaotianzi; Baxter, Daniel

    2016-03-01

    Threshold based direct WIMP dark matter detectors such as the superheated bubble chambers developed by the PICO experiment have demonstrated excellent electron-recoil and alpha discrimination, excellent scalability, ease of change of target fluid, and low cost. However, the nuclear-recoil like backgrounds have been a limiting factor in their dark matter sensitivity. We present a new type of detector, the scintillating bubble chamber, which reads out the scintillation pulse of the scattering events as well as the pressure, temperature, acoustic traces, and bubble images as a conventional bubble chamber does. The event energy provides additional handle to discriminate against the nuclear-recoil like backgrounds. Liquid xenon is chosen as the target fluid in our prototyping detector for its high scintillation yield and suitable vapor pressure which simplifies detector complexity. The detector can be used as an R&D tool to study the backgrounds present in the current PICO bubble chambers or as a prototype for standalone dark matter detectors in the future. Supported by DOE Grant DE-SC0012161.

  15. Pulse height model for deuterated scintillation detectors

    NASA Astrophysics Data System (ADS)

    Wang, Haitang; Enqvist, Andreas

    2015-12-01

    An analytical model of light pulse height distribution for finite deuterated scintillation detectors is created using the impulse approximation. Particularly, the energy distribution of a scattered neutron is calculated based on an existing collision probability scheme for general cylindrical shaped detectors considering double differential cross-sections. The light pulse height distribution is analytically and numerically calculated by convoluting collision sequences with the light output function for an EJ-315 detector from our measurements completed at Ohio University. The model provides a good description of collision histories capturing transferred neutron energy in deuterium-based scintillation materials. The resulting light pulse height distribution details pulse compositions and their corresponding contributions. It shows that probabilities of neutron collision with carbon and deuterium nuclei are comparable, however the light pulse amplitude due to collisions with carbon nuclei is small and mainly located at the lower region of the light pulse distribution axis. The model can explore those neutron interaction events that generate pulses near or below a threshold that would be imposed in measurements. A comparison is made between the light pulse height distributions given by the analytical model and measurements. It reveals a significant probability of a neutron generating a small light pulse due to collisions with carbon nuclei when compared to larger light pulse generated by collisions involving deuterium nuclei. This model is beneficial to understand responses of scintillation materials and pulse compositions, as well as nuclei information extraction from recorded pulses.

  16. A large Scintillating Fibre Tracker for LHCb

    NASA Astrophysics Data System (ADS)

    Greim, R.

    2017-02-01

    The LHCb experiment will be upgraded during LHC Long Shutdown 2 to be able to record data at a higher instantaneous luminosity. The readout rate is currently limited to 1 MHz by the Level 1 trigger. In order to achieve the target integrated luminosity of 50 fb‑1 during LHC Run 3, all subdetectors have to be read out by a 40 MHz trigger-less readout system. Especially, the current tracking detectors downstream of the LHCb dipole magnet suffer from large detector dead times and a small granularity in the Outer Tracker, which consists of proportional straw tubes. Therefore, the Downstream Tracker will be replaced by a Scintillating Fibre Tracker with Silicon Photomultiplier readout. The total sensitive area of 340 m2 is made up of 2.5 m long fibre mats consisting of six staggered layers of 250 μm thin scintillating fibres. The scintillation light created by the charged particles traversing the fibre mats is transported to the fibre ends via total internal reflection and detected by state-of-the-art multi-channel SiPM arrays. This paper presents the detector concept, design, challenges, custom-made readout chips, as well as laboratory and beam test results.

  17. An Approximate Analytic Expression for the Flux Density of Scintillation Light at the Photocathode

    SciTech Connect

    Braverman, Joshua B; Harrison, Mark J; Ziock, Klaus-Peter

    2012-01-01

    The flux density of light exiting scintillator crystals is an important factor affecting the performance of radiation detectors, and is of particular importance for position sensitive instruments. Recent work by T. Woldemichael developed an analytic expression for the shape of the light spot at the bottom of a single crystal [1]. However, the results are of limited utility because there is generally a light pipe and photomultiplier entrance window between the bottom of the crystal and the photocathode. In this study, we expand Woldemichael s theory to include materials each with different indices of refraction and compare the adjusted light spot shape theory to GEANT 4 simulations [2]. Additionally, light reflection losses from index of refraction changes were also taken into account. We found that the simulations closely agree with the adjusted theory.

  18. Metal-loaded organic scintillators for neutrino physics

    NASA Astrophysics Data System (ADS)

    Buck, Christian; Yeh, Minfang

    2016-09-01

    Organic liquid scintillators are used in many neutrino physics experiments of the past and present. In particular for low energy neutrinos when realtime and energy information are required, liquid scintillators have several advantages compared to other technologies. In many cases the organic liquid needs to be loaded with metal to enhance the neutrino signal over background events. Several metal loaded scintillators of the past suffered from chemical and optical instabilities, limiting the performance of these neutrino detectors. Different ways of metal loading are described in the article with a focus on recent techniques providing metal loaded scintillators that can be used under stable conditions for many years even in ton scale experiments. Applications of metal loaded scintillators in neutrino experiments are reviewed and the performance as well as the prospects of different scintillator types are compared.

  19. Metal-loaded organic scintillators for neutrino physics

    DOE PAGES

    Buck, Christian; Yeh, Minfang

    2016-08-03

    Organic liquid scintillators are used in many neutrino physics experiments of the past and present. In particular for low energy neutrinos when realtime and energy information are required, liquid scintillators have several advantages compared to other technologies. In many cases the organic liquid needs to be loaded with metal to enhance the neutrino signal over background events. Several metal loaded scintillators of the past suffered from chemical and optical instabilities, limiting the performance of these neutrino detectors. Different ways of metal loading are described in the article with a focus on recent techniques providing metal loaded scintillators that can bemore » used under stable conditions for many years even in ton scale experiments. Lastly, we review applications of metal loaded scintillators in neutrino experiments and compare the performance as well as the prospects of different scintillator types.« less

  20. Metal-loaded organic scintillators for neutrino physics

    SciTech Connect

    Buck, Christian; Yeh, Minfang

    2016-08-03

    Organic liquid scintillators are used in many neutrino physics experiments of the past and present. In particular for low energy neutrinos when realtime and energy information are required, liquid scintillators have several advantages compared to other technologies. In many cases the organic liquid needs to be loaded with metal to enhance the neutrino signal over background events. Several metal loaded scintillators of the past suffered from chemical and optical instabilities, limiting the performance of these neutrino detectors. Different ways of metal loading are described in the article with a focus on recent techniques providing metal loaded scintillators that can be used under stable conditions for many years even in ton scale experiments. Lastly, we review applications of metal loaded scintillators in neutrino experiments and compare the performance as well as the prospects of different scintillator types.

  1. Separation of scintillation and Cherenkov lights in linear alkyl benzene

    SciTech Connect

    Li, Mohan; Guo, Ziyi; Yeh, Minfang; Wang, Zhe; Chen, Shaomin

    2016-09-11

    To separate scintillation and Cherenkov lights in water-based liquid scintillator detectors is a desired feature for future neutrino and proton decay experiments. Linear alkyl benzene (LAB) is one important ingredient of a water-based liquid scintillator currently under development. In this paper we report on the separation of scintillation and Cherenkov lights observed in an LAB sample. The rise and decay times of the scintillation light are measured to be (7.7±3.0)ns and (36.6±2.4)ns, respectively, while the full width [–3σ, 3σ] of the Cherenkov light is 12 ns and is dominated by the time resolution of the photomultiplier tubes. Here, the scintillation light yield was measured to be(1.01±0.12)×103photons/MeV.

  2. Methods for the continuous production of plastic scintillator materials

    DOEpatents

    Bross, Alan; Pla-Dalmau, Anna; Mellott, Kerry

    1999-10-19

    Methods for producing plastic scintillating material employing either two major steps (tumble-mix) or a single major step (inline-coloring or inline-doping). Using the two step method, the polymer pellets are mixed with silicone oil, and the mixture is then tumble mixed with the dopants necessary to yield the proper response from the scintillator material. The mixture is then placed in a compounder and compounded in an inert gas atmosphere. The resultant scintillator material is then extruded and pelletized or formed. When only a single step is employed, the polymer pellets and dopants are metered into an inline-coloring extruding system. The mixture is then processed under a inert gas atmosphere, usually argon or nitrogen, to form plastic scintillator material in the form of either scintillator pellets, for subsequent processing, or as material in the direct formation of the final scintillator shape or form.

  3. Optical scintillation measurements in a desert environment IV: simulated effects of scintillation on communications links

    NASA Astrophysics Data System (ADS)

    Suite, Michele; Rabinovich, W. S.; Mahon, Rita; Moore, Christopher; Ferraro, Mike; Burris, H. R., Jr.; Thomas, L. M.

    2011-09-01

    Optical scintillation is an effect that limits the performance of many optical systems including imagers and free space optical communication links. The Naval Research Laboratory is undertaking a series of measurement campaigns of optical scintillation in a variety of environments. In December of 2010 measurements were made over a one week period in the desert at China Lake, CA. The NRL TATS system was used to measure time resolved scintillation over a variety of different ranges and terrains. This data has been used to determine fade rate and duration as a function of weather and link margin. Temporal correlation of fades has also been calculated. This data allows simulation of a variety of communication protocols and the effects of those protocols on link throughput. In this paper we present a comparison of different protocols for both direct and retroreflector links.

  4. Synthesis and Screening of Thin Films in the CeCl3-CeBr3 System for Scintillator Applications

    SciTech Connect

    Matson, Dean W.; Graff, Gordon L.; Male, Jonathan L.; Johnson, Bradley R.; Nie, Zimin; Joly, Alan G.; Olsen, Larry C.

    2010-04-02

    Thin film samples of CeCl3, CeBr3, and combinatorial compositions along the CeCl3-CeBr3 join were produced using thermal evaporation, which is being evaluated as a method for rapid screening of new scintillator materials. The combinatorial thin films were shown to be compositionally reproducible from run-to-run within reasonable limitations. Analytical results suggest a continuous variation in the combinatorial samples in terms of their compositions, crystal structures, and luminescence characteristics.

  5. Evaluation of Large Volume SrI2(Eu) Scintillator Detectors

    SciTech Connect

    Sturm, B W; Cherepy, N J; Drury, O B; Thelin, P A; Fisher, S E; Magyar, A F; Payne, S A; Burger, A; Boatner, L A; Ramey, J O; Shah, K S; Hawrami, R

    2010-11-18

    There is an ever increasing demand for gamma-ray detectors which can achieve good energy resolution, high detection efficiency, and room-temperature operation. We are working to address each of these requirements through the development of large volume SrI{sub 2}(Eu) scintillator detectors. In this work, we have evaluated a variety of SrI{sub 2} crystals with volumes >10 cm{sup 3}. The goal of this research was to examine the causes of energy resolution degradation for larger detectors and to determine what can be done to mitigate these effects. Testing both packaged and unpackaged detectors, we have consistently achieved better resolution with the packaged detectors. Using a collimated gamma-ray source, it was determined that better energy resolution for the packaged detectors is correlated with better light collection uniformity. A number of packaged detectors were fabricated and tested and the best spectroscopic performance was achieved for a 3% Eu doped crystal with an energy resolution of 2.93% FWHM at 662keV. Simulations of SrI{sub 2}(Eu) crystals were also performed to better understand the light transport physics in scintillators and are reported. This study has important implications for the development of SrI{sub 2}(Eu) detectors for national security purposes.

  6. Studies of scintillation properties of CaMoO{sub 4} at millikelvin temperatures

    SciTech Connect

    Zhang, X.; Lin, J.; Kraus, H.; Mikhailik, V. B.

    2015-06-15

    Application of CaMoO{sub 4} as a scintillation target in cryogenic rare event searches relies on the understanding of scintillation properties of the material at the temperatures at which these detectors operate. We devised and implemented a detection module with a low-temperature photomultiplier from Hamamatsu (model R8520-06) powered by a Cockcroft-Walton generator. The detector module containing the CaMoO{sub 4} crystal was placed in a {sup 3}He/{sup 4}He dilution refrigerator and used to measure scintillation characteristics of CaMoO{sub 4} in the millikelvin temperature range. At the lowest temperature achieved, the energy resolution of CaMoO{sub 4} for 122 keV γ from a {sup 57}Co source is found to be 30%, and the fast and slow decay constants are 40.6 ± 0.8 μs and 3410 ± 50 μs, respectively. The temperature variation of the CaMoO{sub 4} decay kinetics is discussed in terms of a three-level model of the emission center.

  7. Impact of the Fano Factor on Position and Energy Estimation in Scintillation Detectors

    PubMed Central

    Bora, Vaibhav; Barrett, Harrison H.; Jha, Abhinav K.; Clarkson, Eric

    2015-01-01

    The Fano factor for an integer-valued random variable is defined as the ratio of its variance to its mean. Light from various scintillation crystals have been reported to have Fano factors from sub-Poisson (Fano factor < 1) to super-Poisson (Fano factor > 1). For a given mean, a smaller Fano factor implies a smaller variance and thus less noise. We investigated if lower noise in the scintillation light will result in better spatial and energy resolutions. The impact of Fano factor on the estimation of position of interaction and energy deposited in simple gamma-camera geometries is estimated by two methods - calculating the Cramér-Rao bound and estimating the variance of a maximum likelihood estimator. The methods are consistent with each other and indicate that when estimating the position of interaction and energy deposited by a gamma-ray photon, the Fano factor of a scintillator does not affect the spatial resolution. A smaller Fano factor results in a better energy resolution. PMID:26523069

  8. Scintillating Quantum Dots for Imaging X-rays (SQDIX) for Aircraft Inspection

    NASA Technical Reports Server (NTRS)

    Burke, Eric (Principal Investigator); Williams, Phillip (Principal Investigator); Dehaven, Stan

    2015-01-01

    Scintillation is the process currently employed by conventional x-ray detectors to create x-ray images. Scintillating quantum dots or nano-crystals (StQDs) are a novel, nanometer-scale material that upon excitation by x-rays, re-emit the absorbed energy as visible light. StQDs theoretically have higher output efficiency than conventional scintillating materials and are more environmental friendly. This paper will present the characterization of several critical elements in the use of StQDs that have been performed along a path to the use of this technology in wide spread x-ray imaging. Initial work on the SQDIX system has shown great promise to create state-of-the-art sensors using StQDs as a sensor material. In addition, this work also demonstrates a high degree of promise using StQDs in microstructured fiber optics. Using the microstructured fiber as a light guide could greatly increase the capture efficiency a StQDs based imaging sensor.

  9. Scintillation mechanism of Tb 3+ doped BaY 2F 8

    NASA Astrophysics Data System (ADS)

    de Mello, Ana C. S.; Andrade, Adriano B.; Nakamura, Gerson H. G.; Baldochi, Sonia L.; Valerio, Mário E. G.

    2010-08-01

    In the present work, we report the optical properties of BaY 2F 8 doped with different concentrations of Tb 3+ ions and its potential use as a scintillator in radiation detection. Two types of samples were studied: polycrystalline samples obtained via solid state reaction, and single crystals obtained via the zone melting method under a HF flow. The scintillating properties Tb 3+ doped BaYF were checked by measuring the radioluminescence when excited with X-ray, showing intense emission peaks characteristics of rare-earth ion. Thermoluminescence measurements were done to study the traps competing to inhibit the scintillating process. The radiation damage was evaluated and it was shown that the formation of the absorption bands can be connected to color centers generated by radiation in the matrix. Measurements of DXAS revealed that there is no change in the absorption edge of the dopant during irradiation revealing that the color centers are not connected to changes in the valence of the dopants.

  10. Impact of the Fano Factor on Position and Energy Estimation in Scintillation Detectors.

    PubMed

    Bora, Vaibhav; Barrett, Harrison H; Jha, Abhinav K; Clarkson, Eric

    2015-02-01

    The Fano factor for an integer-valued random variable is defined as the ratio of its variance to its mean. Light from various scintillation crystals have been reported to have Fano factors from sub-Poisson (Fano factor < 1) to super-Poisson (Fano factor > 1). For a given mean, a smaller Fano factor implies a smaller variance and thus less noise. We investigated if lower noise in the scintillation light will result in better spatial and energy resolutions. The impact of Fano factor on the estimation of position of interaction and energy deposited in simple gamma-camera geometries is estimated by two methods - calculating the Cramér-Rao bound and estimating the variance of a maximum likelihood estimator. The methods are consistent with each other and indicate that when estimating the position of interaction and energy deposited by a gamma-ray photon, the Fano factor of a scintillator does not affect the spatial resolution. A smaller Fano factor results in a better energy resolution.

  11. Composite solid-state scintillators for neutron detection

    DOEpatents

    Dai, Sheng; Im, Hee-Jung; Pawel, Michelle D.

    2006-09-12

    Applicant's present invention is a composite scintillator for neutron detection comprising a matrix material fabricated from an inorganic sol-gel precursor solution homogeneously doped with a liquid scintillating material and a neutron absorbing material. The neutron absorbing material yields at least one of an electron, a proton, a triton, an alpha particle or a fission fragment when the neutron absorbing material absorbs a neutron. The composite scintillator further comprises a liquid scintillating material in a self-assembled micelle formation homogeneously doped in the matrix material through the formation of surfactant-silica composites. The scintillating material is provided to scintillate when traversed by at least one of an electron, a proton, a triton, an alpha particle or a fission fragment. The scintillating material is configured such that the matrix material surrounds the micelle formation of the scintillating material. The composite scintillator is fabricated and applied as a thin film on substrate surfaces, a coating on optical fibers or as a glass material.

  12. Ionospheric scintillation observations over Kenyan region - Preliminary results

    NASA Astrophysics Data System (ADS)

    Olwendo, O. J.; Xiao, Yu; Ming, Ou

    2016-11-01

    Ionospheric scintillation refers to the rapid fluctuations in the amplitude and phase of a satellite signal as it passes through small-scale plasma density irregularities in the ionosphere. By analyzing ionospheric scintillation observation datasets from satellite signals such as GPS signals we can study the morphology of ionospheric bubbles. At low latitudes, the diurnal behavior of scintillation is driven by the formation of large-scale equatorial density depletions which form one to two hours after sunset via the Rayleigh-Taylor instability mechanism near the magnetic equator. In this work we present ionospheric scintillation activity over Kenya using data derived from a newly installed scintillation monitor developed by CRIRP at Pwani University (39.78°E, 3.24°S) during the period August to December, 2014. The results reveal the scintillation activity mainly occurs from post-sunset to post-midnight hours, and ceases around 04:00 LT. We also found that the ionospheric scintillation tends to appear at the southwest and northwest of the station. These locations coincide with the southern part of the Equatorial Ionization Anomaly crest over Kenya region. The occurrence of post-midnight L-band scintillation events which are not linked to pre-midnight scintillation observations raises fundamental question on the mechanism and source of electric fields driving the plasma depletion under conditions of very low background electron density.

  13. Development of polystyrene-based scintillation materials and its mechanisms

    NASA Astrophysics Data System (ADS)

    Nakamura, Hidehito; Kitamura, Hisashi; Shinji, Osamu; Saito, Katashi; Shirakawa, Yoshiyuki; Takahashi, Sentaro

    2012-12-01

    Scintillation materials based on polystyrene (PS) have been investigated. Para-terphenyl was employed as a fluorescent molecule (fluor) that functions as a wavelength shifter. A clear increase in photon yield of the scintillation materials relative to the pure PS was observed, which cannot be explained by the conventional theory of scintillation mechanism. Furthermore, the photon yield increased with flour concentration in accordance with a power-law. Here we reveal the emergence of a luminescence of PS-based scintillation materials and demonstrate that their photon yields can be controlled by the fluor concentration.

  14. Plasmonic light yield enhancement of a liquid scintillator

    NASA Astrophysics Data System (ADS)

    Bignell, Lindsey J.; Mume, Eskender; Jackson, Timothy W.; Lee, George P.

    2013-05-01

    We demonstrate modifications to the light yield properties of an organic liquid scintillator due to the localization of the tertiary fluorophore component to the surface of Ag-core silica-shell nanoparticles. We attribute this enhancement to the near-field interaction of Ag nanoparticle plasmons with these fluor molecules. The scintillation light yield enhancement is shown to be equal to the fluorescence enhancement within measurement uncertainties. With a suitable choice of plasmon energy and scintillation fluor, this effect may be used to engineer scintillators with enhanced light yields for radiation detection applications.

  15. Multifrequency equatorial ionospheric scintillations in American and Indian zones

    NASA Technical Reports Server (NTRS)

    Rastogi, R. G.; Aarons, J.; Whitney, H. E.; Mullen, J. P.; Pantoja, J.; Deshpande, M. R.; Vats, H. O.; Chandra, H.; Davies, K.

    1980-01-01

    Amplitude scintillations of 40/41, 140 and 360 MHz transmissions recorded at Huancayo (phase I) and at Ootacamund (phase II) of the ATS-6 program are compared. The scintillations were found to be strongest between 20 and 24 hr LT with another peak around midday. The daytime scintillations do not show a significant seasonal variation at either of these stations. The nighttime scintillations were maximum during December solstices at Huancayo and during equinoxes at Ootacamund and suggested to be due to non-q type of sporadic E following the occurrence of counter-electrojet.

  16. Lanthanide doped strontium-barium cesium halide scintillators

    DOEpatents

    Bizarri, Gregory; Bourret-Courchesne, Edith; Derenzo, Stephen E.; Borade, Ramesh B.; Gundiah, Gautam; Yan, Zewu; Hanrahan, Stephen M.; Chaudhry, Anurag; Canning, Andrew

    2015-06-09

    The present invention provides for a composition comprising an inorganic scintillator comprising an optionally lanthanide-doped strontium-barium, optionally cesium, halide, useful for detecting nuclear material.

  17. Report on radiation exposure of lead-scintillator stack

    SciTech Connect

    Underwood, D.G.

    1990-11-08

    A stack of lead and scintillator was placed in a neutral beam obtained from targeting 800 GeV protons. Small pieces of film containing radiochromic dye were placed adjacent to the layers of scintillator for the purpose of measuring the radiation dose to the scintillator. Our motivation was to calibrate the radiation dose obtainable in this manner for future tests of scintillator for SSC experiments and to relate dose to flux to check absolute normalization for calculations. We also observed several other radiation effects which should be considered for both damage and compensation in a calorimeter.

  18. Plasmonic light yield enhancement of a liquid scintillator

    SciTech Connect

    Bignell, Lindsey J.; Jackson, Timothy W.; Mume, Eskender; Lee, George P.

    2013-05-27

    We demonstrate modifications to the light yield properties of an organic liquid scintillator due to the localization of the tertiary fluorophore component to the surface of Ag-core silica-shell nanoparticles. We attribute this enhancement to the near-field interaction of Ag nanoparticle plasmons with these fluor molecules. The scintillation light yield enhancement is shown to be equal to the fluorescence enhancement within measurement uncertainties. With a suitable choice of plasmon energy and scintillation fluor, this effect may be used to engineer scintillators with enhanced light yields for radiation detection applications.

  19. Observed light yield of scintillation pixels: Extending the two-ray model

    NASA Astrophysics Data System (ADS)

    Kantorski, Igor; Jurkowski, Jacek; Drozdowski, Winicjusz

    2016-09-01

    In this paper we propose an extended, two dimensional model describing the propagation of scintillation photons inside a cuboid crystal until they reach a PMT window. In the simplest approach the model considers two main reasons for light losses: standard absorption obeying the classical Lambert-Beer law and non-ideal reflectivity of the "mummy" covering formed by several layers of Teflon tape wrapping the sample. Results of the model calculations are juxtaposed with experimental data as well as with predictions of an earlier, one dimensional model.

  20. Scintillator assembly for alpha radiation detection and an associated method of making

    DOEpatents

    Lauf, Robert J.; McElhaney, Stephanie A.; Bates, John B.

    1994-01-01

    A scintillator assembly for use in conjunction with a photomultiplier or the like in the detection of alpha radiation utilizes a substrate or transparent yttrium aluminum garnet and a relatively thin film of cerium-doped yttrium aluminum garnet coated upon the substrate. The film material is applied to the substrate in a sputtering process, and the applied film and substrate are annealed to effect crystallization of the film upon the substrate. The resultant assembly provides relatively high energy resolution during use in a detection instrument and is sufficiently rugged for use in field environments.

  1. Scintillator assembly for alpha radiation detection and an associated method of making

    DOEpatents

    Lauf, R.J.; McElhaney, S.A.; Bates, J.B.

    1994-07-26

    A scintillator assembly for use in conjunction with a photomultiplier or the like in the detection of alpha radiation utilizes a substrate or transparent yttrium aluminum garnet and a relatively thin film of cerium-doped yttrium aluminum garnet coated upon the substrate. The film material is applied to the substrate in a sputtering process, and the applied film and substrate are annealed to effect crystallization of the film upon the substrate. The resultant assembly provides relatively high energy resolution during use in a detection instrument and is sufficiently rugged for use in field environments. 4 figs.

  2. Study of radiation hardness of pure CsI crystals for Belle-II calorimeter

    NASA Astrophysics Data System (ADS)

    Boyarintsev, A.; Boyarintseva, Y.; Gektin, A.; Shiran, N.; Shlyakhturov, V.; Taranyuk, V.; Timoshenko, N.; Bobrov, A.; Garmash, A.; Golkovski, M.; Kuzmin, A.; Matvienko, D.; Savrovski, P.; Shebalin, V.; Shwartz, B.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Krumshtein, Z. V.; Nozdrin, A. A.; Olshevsky, A. G.

    2016-03-01

    A study of the radiation hardness of pure CsI crystals 30 cm long was performed with a uniformly absorbed dose of up to 14.3 krad. This study was initiated by the proposed upgrade of the end cap calorimeter of the Belle-II detector, using pure CsI crystals. A set of 14 crystals of truncated pyramid shape used in this study was produced at the Institute for Scintillation Materials NAS from 14 different ingots grown with variations of the growing technology. Interrelationship of crystal scintillation characteristics, radiation hardness and the growing technology was observed.

  3. Recent Developments In Fast Neutron Detection And Multiplicity Counting With Verification With Liquid Scintillator

    SciTech Connect

    Nakae, L; Chapline, G; Glenn, A; Kerr, P; Kim, K; Ouedraogo, S; Prasad, M; Sheets, S; Snyderman, N; Verbeke, J; Wurtz, R

    2011-09-30

    For many years at LLNL, we have been developing time-correlated neutron detection techniques and algorithms for applications such as Arms Control, Threat Detection and Nuclear Material Assay. Many of our techniques have been developed specifically for the relatively low efficiency (a few percent) attainable by detector systems limited to man-portability. Historically, we used thermal neutron detectors (mainly {sup 3}He), taking advantage of the high thermal neutron interaction cross-sections. More recently, we have been investigating the use of fast neutron detection with liquid scintillators, inorganic crystals, and in the near future, pulse-shape discriminating plastics which respond over 1000 times faster (nanoseconds versus tens of microseconds) than thermal neutron detectors. Fast neutron detection offers considerable advantages, since the inherent nanosecond production time-scales of spontaneous fission and neutron-induced fission are preserved and measured instead of being lost by thermalization required for thermal neutron detectors. We are now applying fast neutron technology to the safeguards regime in the form of fast portable digital electronics as well as faster and less hazardous scintillator formulations. Faster detector response times and sensitivity to neutron momentum show promise for measuring, differentiating, and assaying samples that have modest to very high count rates, as well as mixed fission sources like Cm and Pu. We report on measured results with our existing liquid scintillator array, and progress on the design of a nuclear material assay system that incorporates fast neutron detection, including the surprising result that fast liquid scintillator detectors become competitive and even surpass the precision of {sup 3}He-based counters measuring correlated pairs in modest (kg) samples of plutonium.

  4. Search for improved-performance scintillator candidates among the electronic structures of mixed halides

    NASA Astrophysics Data System (ADS)

    Li, Qi; Williams, Richard T.; Burger, Arnold; Adhikari, Rajendra; Biswas, Koushik

    2014-09-01

    The application of advanced theory and modeling techniques has become an essential component to understand material properties and hasten the design and discovery of new ones. This is true for diverse applications. Therefore, current efforts aimed towards finding new scintillator materials are also aligned with this general predictive approach. The need for large scale deployment of efficient radiation detectors requires discovery and development of high-performance, yet low-cost, scintillators. While Tl-doped NaI and CsI are still some of the widely used scintillators, there are promising new developments, for example, Eu-doped SrI2 and Ce-doped LaBr3. The newer candidates have excellent light yield and good energy resolution, but challenges persist in the growth of large single crystals. We will discuss a theoretical basis for anticipating improved proportionality as well as light yield in solid solutions of certain systems, particularly alkali iodides, based on considerations of hot-electron group velocity and thermalization. Solid solutions based on NaI and similar alkali halides are attractive to consider in more detail because the end point compositions are inexpensive and easy to grow. If some of this quality can be preserved while reaping improved light yield and possibly improved proportionality of the mixture, the goal of better performance at the low price of NaI:Tl might be attainable by such a route. Within this context, we will discuss a density functional theory (DFT) based study of two prototype systems: mixed anion NaIxBr1-x and mixed cation NaxK1-xI. Results obtained from these two prototype candidates will lead to further targeted theoretical and experimental search and discovery of new scintillator hosts.

  5. Recent Developments in Fast Neutron Detection and Multiplicity Counting with Liquid Scintillator

    SciTech Connect

    Nakae, L. F.; Chapline, G. F.; Glenn, A. M.; Kerr, P. L.; Kim, K. S.; Ouedraogo, S. A.; Prasad, M. K.; Sheets, S. A.; Snyderman, N. J.; Verbeke, J. M.; Wurtz, R. E.

    2011-12-13

    For many years, LLNL researchers have been developing time-correlated neutron detection techniques and algorithms for applications such as Arms Control, Threat Detection and Nuclear Material Assay. Many of the techniques have been developed specifically for the relatively low efficiency (a few percent) attainable by detector systems limited to man-portability. Historically, thermal neutron detectors (mainly {sup 3}He) were used, taking advantage of the high thermal neutron interaction cross sections. More recently, we have been investigating the use of fast neutron detection with liquid scintillators, inorganic crystals, and in the near future, pulse-shape discriminating plastics that respond over 1000 times faster (ns versus tens of {mu}s) than thermal neutron detectors. Fast neutron detection offers considerable advantages since the inherent ns production timescales of spontaneous fission and neutron-induced fission are preserved and measured instead of being lost by thermalization required for thermal neutron detectors. We are now applying fast neutron technology to the safeguards regime in the form of fast portable digital electronics as well as faster and less hazardous scintillator formulations. Faster detector response times and sensitivity to neutron momentum show promise for measuring, differentiating, and assaying samples that have modest to very high count rates, as well as mixed fission sources like Cm and Pu. We report on measured results with our existing liquid scintillator array and progress on the design of a nuclear material assay system that incorporates fast neutron detection, including the surprising result that fast liquid scintillator detectors become competitive and even surpass the precision of {sup 3}He-based counters measuring correlated pairs in modest (kg) samples of plutonium.

  6. Using MCNP for Compton Scattering Calculations with BGO Scintillators

    NASA Astrophysics Data System (ADS)

    Board, Jeremy; Womble, Phillip; Barzilov, Alexander

    2007-04-01

    Compton scattering is the process wherein photons scatter on the electrons within a material. In a detector, some of these scattered photons leave the detector with only part of their full energy. This creates a continuum which changes the signal to noise ratio with a gamma ray spectrum. For high resolution detectors such as high purity Ge (HPGe) solid state gamma ray detectors, a secondary detector surrounds the HPGe. The purpose of the secondary detector (made of a high Z material) is to detect the scattered photons. When both detectors have coincident photon events, a special circuit stops the data acquisition from acquiring the signal from the HPGe. Our goal is to design the optimal Compton ``suppressor'' using bismuth germinate scintillators for gamma rays whose energies are much larger than 1 MeV. Currently such suppressors are designed for energies less than 2 MeV. We are using the Monte Carlo N-particle code to calculate the amount of photon scattering in the HPGe into geometry of BGO surrounding the HPGe crystal. We are estimating both photon and electron fluence through the volume of BGO.

  7. Scintillator characterization using the LBL Pulsed X-ray Facility

    SciTech Connect

    Moses, W.W.; Derenzo, S.E.; Weber, M.J.; Blankespoor, S.C.; Ho, M.H.; West, A.C.

    1994-10-01

    The authors have developed a bench-top pulsed x-ray system for measuring scintillation properties of compounds in crystal or powdered form. The source is a light-excited x-ray tube that produces 40 x-ray photons (mean energy 18.5 keV) per steradian in each 100 ps fwhm pulse. The repetition rate is adjustable from 0 to 10{sup 7} pulses per second. The fluorescent emanations from the x-ray excited samples are detected with either a sapphire-windowed microchannel plate photomultiplier tube (spectral range 150--650 nm, transit time jitter 40 ps fwhm) or a quartz windowed GaAs(Cs) photomultiplier tube (spectral range 160--930 nm, transit time jitter 4 ns fwhm). Decay time spectra are acquired using a TDC Havina 40 ps fwhm resolution over a 84 ms dynamic range. A computer controlled monochromator can be inserted into the optical path to measure the emission spectrum or wavelength resolved decay time spectrum. A computer controlled sample changer allows up to 64 samples to be measured without intervention.

  8. Linearity for Ca2+-Doped CeBr3 Scintillating Materials

    SciTech Connect

    Guss, Paul

    2014-02-03

    The Remote Sensing Laboratory (RSL) developed an aliovalently calcium-doped cerium tribromide (CeBr3:Ca2+) crystal with 3.2% resolution. RSL completed a crystal assessment, and Sandia National Laboratories calculated the predictive performance and physical characteristics using proven density functional theory (DFT) formalism. Results are reported for the work done to map the detector performance, characteristics, calcium doping concentration, and crystal strength. Preliminary scintillation measurements for this aliovalently calcium-doped CeBr3 scintillator exhibit a slight blue shift in fluorescence emission at 371 nm excitation for CeBr3. The structural, electronic, and optical properties of CeBr3 crystals were investigated using DFT within generalized gradient approximation. The calculated lattice parameters are in good agreement with the experimental data. The energy band structures and density of states were obtained. The optical properties of CeBr3, including the dielectric function, were calculated. Specifically, we report excellent linearity with the aliovalently calcium-doped CeBr3 crystal. Proportionality of light yield is one area of performance in which Ce-doped and Ce-based lanthanide halides excel. Maintaining proportionality is key to producing a strong, high-performance scintillator. Relative light yield proportionality was measured for both doped and undoped samples of CeBr3 to ensure no loss in performance was incurred during doping. The light output and proportionality, however, appear to be similar to CeBr3. There was a reduced yield at low energy. Relative light yield proportionality measurements suggest that dopants do not significantly affect proportionality at higher energies. RSL completed additional testing and evaluation of the new crystal and assessed benchmark spectroscopy measurements. Results, which present energy resolution as a function of energy, are summarized. Typical spectroscopy results using a 137Cs radiation source are shown

  9. Crystal Compton Camera

    SciTech Connect

    Ziock, Klaus-Peter; Braverman, Joshua B.; Harrison, Mark J.; Hornback, Donald Eric; Fabris, Lorenzo; Newby, Jason

    2013-09-26

    Stand-off detection is one of the most important radiation detection capabilities for arms control and the control of illicit nuclear materials. For long range passive detection one requires a large detector and a means of “seeing through” the naturally occurring and varying background radiation, i.e. imaging. Arguably, Compton imaging is the best approach over much of the emission band suitable for long range detection. It provides not only imaging, but more information about the direction of incidence of each detected gamma-ray than the alternate approach of coded-aperture imaging. The directional information allows one to reduce the background and hence improve the sensitivity of a measurement. However, to make an efficient Compton imager requires localizing and measuring the simultaneous energy depositions when gamma-rays Compton scatter and are subsequently captured within a single, large detector volume. This concept has been demonstrated in semi-conductor detectors (HPGe, CZT, Si) but at ~ $1k/cm3 these materials are too expensive to build the large systems needed for standoff detection. Scintillator detectors, such as NaI(Tl), are two orders of magnitude less expensive and possess the energy resolution required to make such an imager. However, they do not currently have the ability to localize closely spaced, simultaneous energy depositions in a single large crystal. In this project we are applying a new technique that should, for the first time ever, allow cubic-millimeter event localization in a bulk scintillator crystal.

  10. Comparing the response of PSD-capable plastic scintillator to standard liquid scintillator

    NASA Astrophysics Data System (ADS)

    Woolf, Richard S.; Hutcheson, Anthony L.; Gwon, Chul; Phlips, Bernard F.; Wulf, Eric A.

    2015-06-01

    This work discusses a test campaign to characterize the response of the recently developed plastic scintillator with pulse shape discrimination (PSD) capabilities (EJ-299-33). PSD is a property exhibited by certain types of scintillating material in which incident stimuli (fast neutrons or γ rays) can be separated by exploiting differences in the scintillation light pulse tail. Detector geometries used were: a 10 cm×10 cm×10 cm cube and a 10-cm diameter×10-cm long cylinder. EJ-301 and EJ-309 liquid scintillators with well-known responses were also tested. The work was conducted at the University of Massachusetts Lowell Van De Graaff accelerator. The facility accelerated protons on a thin Li target to yield quasi-monoenergetic neutrons from the 7Li(p,n)7Be reaction (Q-value: -1.644 MeV). Collimated fast neutrons were obtained by placing detectors behind a neutron spectrometer. Rotating the spectrometer, and thus changing the neutron energy, allowed us to achieve 0.5-3.2 MeV neutrons in 200-300 keV steps. Data were acquired through a flash analog-to-digital converter (ADC) capable of performing digital PSD measurements. By using the PSD technique to separate the neutron events from unwanted γ background, we constructed a pulse height spectrum at each energy. Obtaining a relationship of the relative light output versus energy allowed us to construct the response function for the EJ-299-33 and liquid scintillator. The EJ-299-33 response in terms of electron equivalent energy (Ee.e.) vs. proton equivalent energy (Ep.e.), how it compared with the standard xylene-based EJ-301 (or, NE-213/BC-501 A equivalent) and EJ-309 liquid scintillator response, and how the EJ-301 and EJ-309 compared, are presented. We find that the EJ-299-33 demonstrated a lower light output by up to 40% for <1.0 MeV neutrons; and ranging between a 5-35% reduction for 2.5-3.0 MeV neutrons compared to the EJ-301/309, depending on the scintillator and geometry. Monte Carlo modeling techniques were

  11. Thin-film-based scintillators for hard x-ray microimaging detectors: the ScinTAX Project

    NASA Astrophysics Data System (ADS)

    Rack, A.; Cecilia, A.; Douissard, P.-A.; Dupré, K.; Wesemann, V.; Baumbach, T.; Couchaud, M.; Rochet, X.; Riesemeier, H.; Radtke, M.; Martin, T.

    2014-09-01

    The project ScinTAX developed novel thin scintillating films for the application in high performance X-ray imaging and subsequent introduced new X-ray detectors to the market. To achieve this aim lutetium orthosilicate (LSO) scintillators doped with different activators were grown successfully by liquid phase epitaxy. The high density of LSO (7.4 g/cm3), the effective atomic number (65.2) and the high light yield make this scintillator highly applicable for indirect X-ray detection in which the ionizing radiation is converted into visible light and then registered by a digital detector. A modular indirect detection system has been developed to fully exploit the potential of this thin film scintillator for radiographic and tomographic imaging. The system is compatible for high-resolution imaging with moderate dose as well as adaptable to intense high-dose applications where radiation hard microimaging detectors are required. This proceedings article shall review the achieved performances and technical details on this high-resolution detector system which is now available. A selected example application demonstrates the great potential of the optimized detector system for hard X-ray microimaging, i.e. either to improve image contrast due to the availability of efficient thin crystal films or to reduce the dose to the sample.

  12. Global Morphology of Ionospheric Scintillations II

    DTIC Science & Technology

    1975-03-11

    Fading at Huancayo , Peru 3. Scintillation Contours at 136 MHz for 6 Years Data from Huancayo , Peru 4. Fading on 254 MHz as Observed at Kwajalein 5...Flight Center, NASA Z861-71-239. 8 3.2 Dependence on Magnetic Activity Data from Huancayo , Peru, when analyzed over a long period has shown as a gross...a second increase, that is, after midnight during magnetically disturbed days. 60 HUANCAYO , PERU LES - 6, 254 MHz S1 > 60 -- Kp = 0 - 3 ---Kp=4-9

  13. Thin GSO scintillator for neutron detection

    SciTech Connect

    Reeder, P.L.

    1994-05-01

    The new scintillator cerium-doped gadolinium orthosilicate (GSO -- Gd{sub 2}SiO{sub 5}:Ce) has a light output that is about 20% that of NaI(T1). The enormous cross section of Gd for capture of.thermal neutrons makes GSO a candidate for novel types of neutron.detectors. The characteristic radiations from neutron capture in Gd can be stopped in about 75 {mu}m of GSO. Data obtained from a GSO detector that was about 0.6-mm thick demonstrated that thermal neutrons could easily be detected and that higher energy gamma rays caused minimal interference.

  14. Cherenkov and Scintillation Properties of Cubic Zirconium

    NASA Technical Reports Server (NTRS)

    Christl, M.J.; Adams, J.H.; Parnell, T.A.; Kuznetsov, E.N.

    2008-01-01

    Cubic zirconium (CZ) is a high index of refraction (n =2.17) material that we have investigated for Cherenkov counter applications. Laboratory and proton accelerator tests of an 18cc sample of CZ show that the expected fast Cherenkov response is accompanied by a longer scintillation component that can be separated by pulse shaping. This presents the possibility of novel particle spectrometers which exploits both properties of CZ. Other high index materials being examined for Cherenkov applications will be discussed. Results from laboratory tests and an accelerator exposure will be presented and a potential application in solar energetic particle instruments will be discussed

  15. Measurement of Scintillation and Ionization Yield and Scintillation Pulse Shape from Nuclear Recoils in Liquid Argon

    DOE PAGES

    Cao, H.

    2015-05-26

    We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We also report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median applied electric fields from 0more » to 970 V/cm. For the ionization yields, we report measurements from 16.9 to 57.3 keV and for electric fields from 96.4 to 486 V/cm. Furthermore, we report the observation of an anticorrelation between scintillation and ionization from nuclear recoils, which is similar to the anticorrelation between scintillation and ionization from electron recoils. Assuming that the energy loss partitions into excitons and ion pairs from 83mKr internal conversion electrons is comparable to that from 207Bi conversion electrons, we obtained the numbers of excitons (Nex) and ion pairs (Ni) and their ratio (Nex/Ni) produced by nuclear recoils from 16.9 to 57.3 keV. Motivated by arguments suggesting direction sensitivity in LAr-TPC signals due to columnar recombination, a comparison of the light and charge yield of recoils parallel and perpendicular to the applied electric field is presented for the first time.« less

  16. Measurement of scintillation and ionization yield and scintillation pulse shape from nuclear recoils in liquid argon

    NASA Astrophysics Data System (ADS)

    Cao, H.; Alexander, T.; Aprahamian, A.; Avetisyan, R.; Back, H. O.; Cocco, A. G.; Dejongh, F.; Fiorillo, G.; Galbiati, C.; Grandi, L.; Guardincerri, Y.; Kendziora, C.; Lippincott, W. H.; Love, C.; Lyons, S.; Manenti, L.; Martoff, C. J.; Meng, Y.; Montanari, D.; Mosteiro, P.; Olvitt, D.; Pordes, S.; Qian, H.; Rossi, B.; Saldanha, R.; Sangiorgio, S.; Siegl, K.; Strauss, S. Y.; Tan, W.; Tatarowicz, J.; Walker, S.; Wang, H.; Watson, A. W.; Westerdale, S.; Yoo, J.; Scene Collaboration

    2015-05-01

    We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median applied electric fields from 0 to 970 V /cm . For the ionization yields, we report measurements from 16.9 to 57.3 keV and for electric fields from 96.4 to 486 V /cm . We also report the observation of an anticorrelation between scintillation and ionization from nuclear recoils, which is similar to the anticorrelation between scintillation and ionization from electron recoils. Assuming that the energy loss partitions into excitons and ion pairs from Krm83 internal conversion electrons is comparable to that from 207Bi conversion electrons, we obtained the numbers of excitons (Nex) and ion pairs (Ni) and their ratio (Nex/Ni ) produced by nuclear recoils from 16.9 to 57.3 keV. Motivated by arguments suggesting direction sensitivity in LAr-TPC signals due to columnar recombination, a comparison of the light and charge yield of recoils parallel and perpendicular to the applied electric field is presented for the first time.

  17. Measurement of Scintillation and Ionization Yield and Scintillation Pulse Shape from Nuclear Recoils in Liquid Argon

    SciTech Connect

    Cao, H.

    2015-05-26

    We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We also report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median applied electric fields from 0 to 970 V/cm. For the ionization yields, we report measurements from 16.9 to 57.3 keV and for electric fields from 96.4 to 486 V/cm. Furthermore, we report the observation of an anticorrelation between scintillation and ionization from nuclear recoils, which is similar to the anticorrelation between scintillation and ionization from electron recoils. Assuming that the energy loss partitions into excitons and ion pairs from 83mKr internal conversion electrons is comparable to that from 207Bi conversion electrons, we obtained the numbers of excitons (Nex) and ion pairs (Ni) and their ratio (Nex/Ni) produced by nuclear recoils from 16.9 to 57.3 keV. Motivated by arguments suggesting direction sensitivity in LAr-TPC signals due to columnar recombination, a comparison of the light and charge yield of recoils parallel and perpendicular to the applied electric field is presented for the first time.

  18. Microprocessor-based single particle calibration of scintillation counter

    NASA Technical Reports Server (NTRS)

    Mazumdar, G. K. D.; Pathak, K. M.

    1985-01-01

    A microprocessor-base set-up is fabricated and tested for the single particle calibration of the plastic scintillator. The single particle response of the scintillator is digitized by an A/D converter, and a 8085 A based microprocessor stores the pulse heights. The digitized information is printed. Facilities for CRT display and cassette storing and recalling are also made available.

  19. Applications for New Scintillator Technologies in Gamma Ray Astronomy

    NASA Astrophysics Data System (ADS)

    McConnell, Mark L.; Bloser, Peter F.; Legere, Jason; Ryan, James M.

    2016-10-01

    Scintillators have long been used for probing the high energy universe. The reliability and low cost of scintillator-PMT detectors have made them the de facto standard for experiments on high altitude balloons and in orbiting satellites. New scintillators and new readout technologies offer important opportunities for more capable experiments. Recent scintillator developments include faster signals, increased light output, improved energy resolution, and better handling characteristics. Although PMTs remain effective for scintillator readout, new technologies offer more compact, rugged devices with much lower operational voltages. The adoption of these technologies is not without its difficulties, especially for space applications, where the technology readiness level can be an important consideration. To illustrate these issues, we will discuss the use of scintillators in Compton imaging experiments. At energies from about 500 keV to 30 MeV, Compton telescopes are the most effective means of imaging the gamma ray sky. To date, the only Compton telescope that has flown in space was the COMPTEL instrument on NASA's Compton Gamma Ray Observatory (CGRO). CGRO, launched in 1991 and de-orbited in 2000, was based entirely on the use of technologies from the 1980’s. We have been working on an improved Compton telescope design, called the Advanced Scintillator Compton Telescope (ASCOT). It is much like COMPTEL, but utilizes up-to-date scintillator and readout technologies.

  20. Scintillation of nonuniformly correlated beams in atmospheric turbulence.

    PubMed

    Gu, Yalong; Gbur, Greg

    2013-05-01

    We investigated the scintillation properties of nonuniformly correlated (NUC) beams in atmospheric turbulence and have shown that NUC beams can not only have lower scintillation but also higher intensity than Gaussian-Schell model beams and even higher intensity than coherent Gaussian beams over certain propagation distances.