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Sample records for rayleigh scattering

  1. Rayleigh Scattering.

    ERIC Educational Resources Information Center

    Young, Andrew T.

    1982-01-01

    The correct usage of such terminology as "Rayleigh scattering,""Rayleigh lines,""Raman lines," and "Tyndall scattering" is resolved during an historical excursion through the physics of light-scattering by gas molecules. (Author/JN)

  2. Rayleigh Scattering Diagnostics Workshop

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard (Compiler)

    1996-01-01

    The Rayleigh Scattering Diagnostics Workshop was held July 25-26, 1995 at the NASA Lewis Research Center in Cleveland, Ohio. The purpose of the workshop was to foster timely exchange of information and expertise acquired by researchers and users of laser based Rayleigh scattering diagnostics for aerospace flow facilities and other applications. This Conference Publication includes the 12 technical presentations and transcriptions of the two panel discussions. The first panel was made up of 'users' of optical diagnostics, mainly in aerospace test facilities, and its purpose was to assess areas of potential applications of Rayleigh scattering diagnostics. The second panel was made up of active researchers in Rayleigh scattering diagnostics, and its purpose was to discuss the direction of future work.

  3. Rayleigh scattering. [molecular scattering terminology redefined

    NASA Technical Reports Server (NTRS)

    Young, A. T.

    1981-01-01

    The physical phenomena of molecular scattering are examined with the objective of redefining the confusing terminology currently used. The following definitions are proposed: molecular scattering consists of Rayleigh and vibrational Raman scattering; the Rayleigh scattering consists of rotational Raman lines and the central Cabannes line; the Cabannes line is composed of the Brillouin doublet and the central Gross or Landau-Placzek line. The term 'Rayleigh line' should never be used.

  4. Interferometric Rayleigh Scattering Measurement System

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel (Inventor); Danehy, Paul M. (Inventor); Lee, Joseph W. (Inventor)

    2008-01-01

    A method and apparatus for performing simultaneous multi-point measurements of multiple velocity components in a gas flow is described. Pulses of laser light are directed to a measurement region of unseeded gas to produce Rayleigh or Mie scattered light in a plurality of directions. The Rayleigh or Mie scattered light is collected from multiple directions and combined in a single collimated light beam. The Rayleigh or Mie scattered light is then mixed together with a reference laser light before it is passed through a single planar Fabry-Perot interferometer for spectral analysis. At the output of the interferometer, a high-sensitivity CCD camera images the interference fringe pattern. This pattern contains the spectral and spatial information from both the Rayleigh scattered light and the reference laser light. Interferogram processing software extracts and analyzes spectral profiles to determine the velocity components of the gas flow at multiple points in the measurement region. The Rayleigh light rejected by the interferometer is recirculated to increase the accuracy and the applicability of the method for measurements at high temperatures without requiring an increase in the laser energy.

  5. Rayleigh Scattering by Helium in Stellar Atmospheres

    NASA Astrophysics Data System (ADS)

    Fišák, J.; Kubát, J.; Krtička, J.

    2017-02-01

    We study the influence of Rayleigh scattering by helium on synthetic spectra and stellar atmosphere models. Rayleigh scattering by helium is often neglected in hot star atmosphere models. This approximation is justified by the small population of helium in stars with solar composition (about 10% by number) and lower Rayleigh scattering total cross section of helium with respect to neutral hydrogen. However, for stars with large helium abundances Rayleigh scattering by helium can be a significant opacity source.

  6. Rayleigh, Raman and particulate scattering

    NASA Technical Reports Server (NTRS)

    Cochran, W. D.

    1982-01-01

    Analysis of the visible and near infrared spectra of planetary atmospheres and the multiple scattering of photons within the atmosphere are discussed. Photons detected within the spectral region are solar photons which were scattered by the gas and particles in the planetary atmosphere. An example is given for the incident and emitted fluxes for a hypothetical planet with an effective temperature of 100 K. The absorption spectrum of the planetary atmosphere is discussed in terms of the various scattering processes photons undergo within the atmosphere. Three different physical processes are considered. Rayleigh scattering and Raman scattering by the gas molecules, and scattering by any cloud or dust aerosol particles in the atmosphere. The physics of each of these processes is examined.

  7. Blue Skies, Coffee Creamer, and Rayleigh Scattering

    ERIC Educational Resources Information Center

    Liebl, Michael

    2010-01-01

    The first physical explanation of Earths blue sky was fashioned in 1871 by Lord Rayleigh. Many discussions of Rayleigh scattering and approaches to studying it both in and out of the classroom are available. Rayleigh scattering accounts for the blue color of the sky and the orange/red color of the Sun near sunset and sunrise, and a number of…

  8. Improvement in Rayleigh Scattering Measurement Accuracy

    NASA Technical Reports Server (NTRS)

    Fagan, Amy F.; Clem, Michelle M.; Elam, Kristie A.

    2012-01-01

    Spectroscopic Rayleigh scattering is an established flow diagnostic that has the ability to provide simultaneous velocity, density, and temperature measurements. The Fabry-Perot interferometer or etalon is a commonly employed instrument for resolving the spectrum of molecular Rayleigh scattered light for the purpose of evaluating these flow properties. This paper investigates the use of an acousto-optic frequency shifting device to improve measurement accuracy in Rayleigh scattering experiments at the NASA Glenn Research Center. The frequency shifting device is used as a means of shifting the incident or reference laser frequency by 1100 MHz to avoid overlap of the Rayleigh and reference signal peaks in the interference pattern used to obtain the velocity, density, and temperature measurements, and also to calibrate the free spectral range of the Fabry-Perot etalon. The measurement accuracy improvement is evaluated by comparison of Rayleigh scattering measurements acquired with and without shifting of the reference signal frequency in a 10 mm diameter subsonic nozzle flow.

  9. Stimulated thermal Rayleigh scattering in optical fibers.

    PubMed

    Dong, Liang

    2013-02-11

    Recently, mode instability was observed in optical fiber lasers at high powers, severely limiting power scaling for single-mode outputs. Some progress has been made towards understanding the underlying physics. A thorough understanding of the effect is critical for continued progress of this very important technology area. Mode instability in optical fibers is, in fact, a manifestation of stimulated thermal Rayleigh scattering. In this work, a quasi-closed-form solution for the nonlinear coupling coefficient is found for stimulated thermal Rayleigh scattering in optical fibers. The results help to significantly improve understanding of mode instability.

  10. Rayleigh scattering measurements of several fluorocarbon gases.

    PubMed

    Zadoo, Serena; Thompson, Jonathan E

    2011-11-01

    Integrating nephelometers are commonly used to monitor airborne particulate matter. However, they must be calibrated prior to use. The Rayleigh scattering coefficients (b(RS), Mm(-1)), scattering cross sections (σ(RS), cm(2)), and Rayleigh multipliers for tetrafluoromethane (R-14), sulfur hexafluoride, pentafluoroethane (HFC-125), hexafluoropropene (HFC-216), 1,1,1,2,3,3,3,-heptafluoropropane (HFC-227ea), and octafluorocyclobutane (C-318) are reported from measurements made using a Radiance Research M903 integrating nephelometer operating at λ = 530 nm and calibration with gases of known scattering constants. Rayleigh multipliers (±90% conf. int.) were found to be 2.6 ± 0.5, 6.60 ± 0.07, 7.5 ± 1, 14.8 ± 0.9, 15.6 ± 0.5, and 22.3 ± 0.8 times that of air, respectively. To the best of our knowledge, these are the first reported values for R-14, HFC-216, HFC-125, and C-318. Experimental accuracy is supported through measurements of values for SF(6) and HFC-227ea which agree to within 3% of previous literature reports. In addition to documenting fundamental Rayleigh scattering data for the first time, the information presented within will find use for calibration of optical scattering sensors such as integrating nephelometers.

  11. Simultaneous CARS and Interferometric Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Danehy, Paul M.; Grinstead, Keith D., Jr.; Tedder, Sarah; Cutler, Andrew D.

    2006-01-01

    This paper reports for the first time the combination of a dual-pump coherent anti-Stokes Raman scattering system with an interferometric Rayleigh scattering system (CARS - IRS) to provide time-resolved simultaneous measurement of multiple properties in combustion flows. The system uses spectrally narrow green (seeded Nd:YAG at 532 nm) and yellow (552.9 nm) pump beams and a spectrally-broad red (607 nm) beam as the Stokes beam. A spectrometer and a planar Fabry-Perot interferometer used in the imaging mode are used to record the spectrally broad CARS spectra and the spontaneous Rayleigh scattering spectra, respectively. Time-resolved simultaneous measurement of temperature, absolute mole fractions of N2, O2, and H2, and two components of velocity in a Hencken burner flame were performed to demonstrate the technique.

  12. Molecular filtered Rayleigh scattering applied to combustion

    NASA Astrophysics Data System (ADS)

    Elliott, Gregory S.; Glumac, Nick; Carter, Campbell D.

    2001-04-01

    Molecular filtered Rayleigh scattering (FRS), employing an iodine vapour filter and an injection-seeded Nd:YAG laser, was utilized to measure instantaneous and average temperature fields in combustion environments. With FRS thermometry, the vapour within the cell strongly absorbs background scattering from surfaces and particles, while much of the Doppler-broadened Rayleigh scattering is not absorbed by the iodine transition; the gas temperature can then be deduced from the measured transmission of the molecular Rayleigh scattering. For demonstration purposes and to evaluate the accuracy of the technique, we employed a near-adiabatic hydrogen-air flame. The accuracy of the FRS measurements was investigated by comparing FRS-derived temperatures with those (1) calculated assuming adiabatic equilibrium conditions and (2) recorded with the CARS (coherent anti-Stokes Raman spectroscopy) technique. For the hydrogen-air flames, the FRS method gave temperatures within 2% of the expected value. The FRS thermometry instrument was then applied to a stagnation-flow, premixed methane-air flame; images recorded here demonstrate the utility of the FRS method for temperature imaging, particularly near surfaces. In this flow field, we compared the FRS temperatures with those from a one-dimensional model and investigated the radial extent of the uniform temperature region, to assess the assumption of one-dimensionality. In addition, we demonstrated the feasibility of simultaneous measurements of the temperature and velocity fields, the latter derived from the particle image velocimetry technique.

  13. Rayleigh wave scattering from sessile droplets

    NASA Astrophysics Data System (ADS)

    Quintero, R.; Simonetti, F.

    2013-10-01

    Radiation of energy by large-amplitude leaky Rayleigh waves is regarded as one of the key physical mechanisms regulating the actuation and manipulation of droplets in surface acoustic wave (SAW) microfluidic devices. The interaction between a SAW and a droplet is highly complex and is presently the subject of extensive research. This paper investigates the existence of an additional interaction mechanism based on the propagation of quasi-Stoneley waves inside sessile droplets deposited on a solid substrate. In contrast with the leaky Rayleigh wave, the energy of the Stoneley wave is confined within a thin fluid layer in contact with the substrate. The hypothesis is confirmed by three-dimensional finite element simulations and ultrasonic scattering experiments measuring the reflection of Rayleigh waves from droplets of different diameters. Moreover, real-time monitoring of the droplet evaporation process reveals a clear correlation between the droplet contact angle and the spectral information of the reflected Rayleigh signal, thus paving the way for ultrasonic measurements of surface tension.

  14. Filtered Rayleigh Scattering Measurements in a Buoyant Flow Field

    DTIC Science & Technology

    2008-03-01

    John William Strutt , the third Baron of Rayleigh , or more commonly known as Lord Rayleigh , was the first to offer a correct explanation of the...FILTERED RAYLEIGH SCATTERING MEASUREMENTS IN A BUOYANT FLOW FIELD         THESIS       Steven Michael Meents, Captain, USAF...AFIT/GAE/ENY/08-M22 FILTERED RAYLEIGH SCATTERING MEASUREMENTS IN A BUOYANT FLOW FIELD THESIS Presented to the Faculty Department of Aeronautics

  15. Generalized Rayleigh scattering. I. Basic theory.

    NASA Astrophysics Data System (ADS)

    Ivanov, V. V.

    1995-11-01

    The classsical problem of multiple molecular (in particular, Rayleigh) scattering in plane-parallel atmospheres is considered from a somewhat broader viewpoint than usual. The general approach and ideology are borrowed from non-LTE line formation theory. The main emphasis is on the depth dependence of the corresponding source matrix rather than on the emergent radiation. We study the azimuth-averaged radiation field of polarized radiation in a semi-infinite atmosphere with embedded primary sources. The corresponding 2x2 phase matrix of molecular scattering is P=(1-W) P_I_+W P_R_, where P_I_ and P_R_ are the phase matrices of the scalar isotropic scattering and of the Rayleigh scattering, respectively, and W is the depolarization parameter. Contrary to the usual assumption that W{in}[0,1], we assume W{in} [0,{infinity}) and call this generalized Rayleigh scattering (GRS). Using the factorization of P which is intimately related to its diadic expansion, we reduce the problem to an integral equation for the source matrix S(τ) with a matrix displacement kernel. In operator form this equation is S={LAMBDA}S+S^*^, where {LAMBDA} is the matrix {LAMBDA}-operator and S^*^ is the primary source term. This leads to a new concept, the matrix albedo of single scattering λ =diag(λ_I_,λ_Q_), where λ_I_ is the usual (scalar) single scattering albedo and λ_Q_=0.7Wλ_I_. Its use enables one to formulate matrix equivalents of many of the results of the scalar theory in exactly the same form as in the scalar case. Of crucial importance is the matrix equivalent of the sqrt(ɛ) law of the scalar theory. Another useful new concept is the λ-plane, i.e., the plane with the axes (λ_I_,λ_Q_). Systematic use of the matrix sqrt(ɛ) law and of the λ-plane proved to be a useful instrument in classifying various limiting and particular cases of GRS and in discussing numerical data on the matrix source functions (to be given in Paper II of the series).

  16. Spontaneous inelastic Rayleigh scattering in optical fibers.

    PubMed

    Okusaga, Olukayode; Cahill, James P; Docherty, Andrew; Menyuk, Curtis R; Zhou, Weimin

    2013-02-15

    Rayleigh scattering (RS) adds noise to signals that are transmitted over optical fibers and other optical waveguides. This noise can be the dominant noise source in a range between 10 Hz and 100 kHz from the carrier and can seriously degrade the performance of optical systems that require low close-in noise. Using heterodyne techniques, we demonstrate that the backscattered close-in noise spectrum in optical fibers is symmetric about the carrier and grows linearly with both input power and fiber length. These results indicate that the RS is spontaneous and is due to finite-lifetime thermal fluctuations in the glass.

  17. Rayleigh scattering of linear alkylbenzene in large liquid scintillator detectors.

    PubMed

    Zhou, Xiang; Liu, Qian; Wurm, Michael; Zhang, Qingmin; Ding, Yayun; Zhang, Zhenyu; Zheng, Yangheng; Zhou, Li; Cao, Jun; Wang, Yifang

    2015-07-01

    Rayleigh scattering poses an intrinsic limit for the transparency of organic liquid scintillators. This work focuses on the Rayleigh scattering length of linear alkylbenzene (LAB), which will be used as the solvent of the liquid scintillator in the central detector of the Jiangmen Underground Neutrino Observatory. We investigate the anisotropy of the Rayleigh scattering in LAB, showing that the resulting Rayleigh scattering length will be significantly shorter than reported before. Given the same overall light attenuation, this will result in a more efficient transmission of photons through the scintillator, increasing the amount of light collected by the photosensors and thereby the energy resolution of the detector.

  18. Rayleigh scattering of linear alkylbenzene in large liquid scintillator detectors

    SciTech Connect

    Zhou, Xiang Zhang, Zhenyu; Liu, Qian; Zheng, Yangheng; Wurm, Michael; Zhang, Qingmin; Ding, Yayun; Zhou, Li; Cao, Jun; Wang, Yifang

    2015-07-15

    Rayleigh scattering poses an intrinsic limit for the transparency of organic liquid scintillators. This work focuses on the Rayleigh scattering length of linear alkylbenzene (LAB), which will be used as the solvent of the liquid scintillator in the central detector of the Jiangmen Underground Neutrino Observatory. We investigate the anisotropy of the Rayleigh scattering in LAB, showing that the resulting Rayleigh scattering length will be significantly shorter than reported before. Given the same overall light attenuation, this will result in a more efficient transmission of photons through the scintillator, increasing the amount of light collected by the photosensors and thereby the energy resolution of the detector.

  19. Rayleigh Scattering for Measuring Flow in a Nozzle Testing Facility

    NASA Technical Reports Server (NTRS)

    Gomez, Carlos R.; Panda, Jayanta

    2006-01-01

    A molecular Rayleigh-scattering-based air-density measurement system was built in a large nozzle-and-engine-component test facility for surveying supersonic plumes from jet-engine exhaust. A molecular Rayleigh-scattering-based air-density measurement system was built in a large nozzle-and-enginecomponent test facility for surveying supersonic plumes from jet-engine exhaust

  20. Technical Report: Rayleigh Scattering Combustion Diagnostic

    SciTech Connect

    Adams, Wyatt; Hecht, Ethan

    2015-07-29

    A laser Rayleigh scattering (LRS) temperature diagnostic was developed over 8 weeks with the goal of studying oxy-combustion of pulverized coal char in high temperature reaction environments with high concentrations of carbon dioxide. Algorithms were developed to analyze data collected from the optical diagnostic system and convert the information to temperature measurements. When completed, the diagnostic will allow for the kinetic gasification rates of the oxy-combustion reaction to be obtained, which was previously not possible since the high concentrations of high temperature CO2 consumed thermocouples that were used to measure flame temperatures inside the flow reactor where the combustion and gasification reactions occur. These kinetic rates are important for studying oxycombustion processes suitable for application as sustainable energy solutions.

  1. Rayleigh scattering: blue sky thinking for future CMB observations

    SciTech Connect

    Lewis, Antony

    2013-08-01

    Rayleigh scattering from neutral hydrogen during and shortly after recombination causes the CMB anisotropies to be significantly frequency dependent at high frequencies. This may be detectable with Planck, and would be a strong signal in any future space-based CMB missions. The later peak of the Rayleigh visibility compared to Thomson scattering gives an increased large-scale CMB polarization signal that is a greater than 4% effect for observed frequencies ν ∼> 500GHz. There is a similar magnitude suppression on small scales from additional damping. Due to strong correlation between the Rayleigh and primary signal, measurement of the Rayleigh component is limited by noise and foregrounds, not cosmic variance of the primary CMB, and should observable over a wide range of angular scales at frequencies 200GHz ∼< ν ∼< 800GHz. I give new numerical calculations of the temperature and polarization power spectra, and show that future CMB missions could measure the temperature Rayleigh cross-spectrum at high precision, detect the polarization from Rayleigh scattering, and also accurately determine the cross-spectra between the Rayleigh temperature signal and primary polarization. The Rayleigh scattering signal may provide a powerful consistency check on recombination physics. In principle it can be used to measure additional horizon-scale primordial perturbation modes at recombination, and distinguish a significant tensor mode B-polarization signal from gravitational lensing at the power spectrum level.

  2. Correction of Rayleigh Scattering Effects in Cloud Optical Thickness Retrievals

    NASA Technical Reports Server (NTRS)

    Wang, Meng-Hua; King, Michael D.

    1997-01-01

    We present results that demonstrate the effects of Rayleigh scattering on the 9 retrieval of cloud optical thickness at a visible wavelength (0.66 Am). The sensor-measured radiance at a visible wavelength (0.66 Am) is usually used to infer remotely the cloud optical thickness from aircraft or satellite instruments. For example, we find that without removing Rayleigh scattering effects, errors in the retrieved cloud optical thickness for a thin water cloud layer (T = 2.0) range from 15 to 60%, depending on solar zenith angle and viewing geometry. For an optically thick cloud (T = 10), on the other hand, errors can range from 10 to 60% for large solar zenith angles (0-60 deg) because of enhanced Rayleigh scattering. It is therefore particularly important to correct for Rayleigh scattering contributions to the reflected signal from a cloud layer both (1) for the case of thin clouds and (2) for large solar zenith angles and all clouds. On the basis of the single scattering approximation, we propose an iterative method for effectively removing Rayleigh scattering contributions from the measured radiance signal in cloud optical thickness retrievals. The proposed correction algorithm works very well and can easily be incorporated into any cloud retrieval algorithm. The Rayleigh correction method is applicable to cloud at any pressure, providing that the cloud top pressure is known to within +/- 100 bPa. With the Rayleigh correction the errors in retrieved cloud optical thickness are usually reduced to within 3%. In cases of both thin cloud layers and thick ,clouds with large solar zenith angles, the errors are usually reduced by a factor of about 2 to over 10. The Rayleigh correction algorithm has been tested with simulations for realistic cloud optical and microphysical properties with different solar and viewing geometries. We apply the Rayleigh correction algorithm to the cloud optical thickness retrievals from experimental data obtained during the Atlantic

  3. Effects of Rayleigh scattering on the CMB and cosmic structure

    NASA Astrophysics Data System (ADS)

    Alipour, Elham; Sigurdson, Kris; Hirata, Christopher M.

    2015-04-01

    During and after recombination, in addition to Thomson scattering with free electrons, photons also couple to neutral hydrogen and helium atoms through Rayleigh scattering. This coupling influences both cosmic microwave background (CMB) anisotropies and the distribution of matter in the Universe. The frequency dependence of the Rayleigh cross section breaks the thermal nature of CMB temperature and polarization anisotropies and effectively doubles the number of variables needed to describe CMB intensity and polarization statistics, while the additional atomic coupling changes the matter distribution and the lensing of the CMB. We introduce a new method to capture the effects of Rayleigh scattering on cosmological power spectra. Rayleigh scattering modifies CMB temperature and polarization anisotropies at the ˜1 % level at 35 GHz (scaling ∝ν4 ), and modifies matter correlations by as much as ˜0.3 %. We show the Rayleigh signal, especially the cross-spectra between the thermal (Rayleigh) E -polarization and Rayleigh (thermal) intensity signal, may be detectable with future CMB missions even in the presence of foregrounds, and how this new information might help to better constrain the cosmological parameters.

  4. In situ Characterization of Nanoparticles Using Rayleigh Scattering

    PubMed Central

    Santra, Biswajit; Shneider, Mikhail N.; Car, Roberto

    2017-01-01

    We report a theoretical analysis showing that Rayleigh scattering could be used to monitor the growth of nanoparticles under arc discharge conditions. We compute the Rayleigh scattering cross sections of the nanoparticles by combining light scattering theory for gas-particle mixtures with calculations of the dynamic electronic polarizability of the nanoparticles. We find that the resolution of the Rayleigh scattering probe is adequate to detect nanoparticles as small as C60 at the expected concentrations of synthesis conditions in the arc periphery. Larger asymmetric nanoparticles would yield brighter signals, making possible to follow the evolution of the growing nanoparticle population from the evolution of the scattered intensity. Observable spectral features include characteristic resonant behaviour, shape-dependent depolarization ratio, and mass-dependent line shape. Direct observation of nanoparticles in the early stages of growth with unobtrusive laser probes should give insight on the particle formation mechanisms and may lead to better-controlled synthesis protocols. PMID:28071715

  5. In situ Characterization of Nanoparticles Using Rayleigh Scattering.

    PubMed

    Santra, Biswajit; Shneider, Mikhail N; Car, Roberto

    2017-01-10

    We report a theoretical analysis showing that Rayleigh scattering could be used to monitor the growth of nanoparticles under arc discharge conditions. We compute the Rayleigh scattering cross sections of the nanoparticles by combining light scattering theory for gas-particle mixtures with calculations of the dynamic electronic polarizability of the nanoparticles. We find that the resolution of the Rayleigh scattering probe is adequate to detect nanoparticles as small as C60 at the expected concentrations of synthesis conditions in the arc periphery. Larger asymmetric nanoparticles would yield brighter signals, making possible to follow the evolution of the growing nanoparticle population from the evolution of the scattered intensity. Observable spectral features include characteristic resonant behaviour, shape-dependent depolarization ratio, and mass-dependent line shape. Direct observation of nanoparticles in the early stages of growth with unobtrusive laser probes should give insight on the particle formation mechanisms and may lead to better-controlled synthesis protocols.

  6. In situ Characterization of Nanoparticles Using Rayleigh Scattering

    NASA Astrophysics Data System (ADS)

    Santra, Biswajit; Shneider, Mikhail N.; Car, Roberto

    2017-01-01

    We report a theoretical analysis showing that Rayleigh scattering could be used to monitor the growth of nanoparticles under arc discharge conditions. We compute the Rayleigh scattering cross sections of the nanoparticles by combining light scattering theory for gas-particle mixtures with calculations of the dynamic electronic polarizability of the nanoparticles. We find that the resolution of the Rayleigh scattering probe is adequate to detect nanoparticles as small as C60 at the expected concentrations of synthesis conditions in the arc periphery. Larger asymmetric nanoparticles would yield brighter signals, making possible to follow the evolution of the growing nanoparticle population from the evolution of the scattered intensity. Observable spectral features include characteristic resonant behaviour, shape-dependent depolarization ratio, and mass-dependent line shape. Direct observation of nanoparticles in the early stages of growth with unobtrusive laser probes should give insight on the particle formation mechanisms and may lead to better-controlled synthesis protocols.

  7. Electric field autocorrelation functions for beginning multiple rayleigh scattering.

    PubMed

    Lock, J A

    2001-08-20

    The polarization-resolved electric field autocorrelation function for p-order scattering was derived from the order-of-scattering solution of the exact equations for electromagnetic multiple Rayleigh scattering and was calculated for 2 scattering-angle dependence of the p-order autocorrelation function approximately decoupled from the delay-time dependence for p ? 3. The polarization-channel and the scattering-angle dependence were analytically calculated, and the delay-time dependence was analytically approximated. The resulting analytical model for the polarization-resolved autocorrelation function for beginning multiple Rayleigh scattering was then tested against experimental autocorrelation data. The data were found to be well fitted by the model.

  8. Electric Field Autocorrelation Functions for Beginning Multiple Rayleigh Scattering

    NASA Astrophysics Data System (ADS)

    Lock, James A.

    2001-08-01

    The polarization-resolved electric field autocorrelation function for p -order scattering was derived from the order-of-scattering solution of the exact equations for electromagnetic multiple Rayleigh scattering and was calculated for 2 p 6 for particles undergoing diffusive motion in an idealized sample cell. It was found that the polarization-channel and the scattering-angle dependence of the p -order autocorrelation function approximately decoupled from the delay-time dependence for p ~ 3 . The polarization-channel and the scattering-angle dependence were analytically calculated, and the delay-time dependence was analytically approximated. The resulting analytical model for the polarization-resolved autocorrelation function for beginning multiple Rayleigh scattering was then tested against experimental autocorrelation data. The data were found to be well fitted by the model.

  9. Multiple-Point Mass Flux Measurement System Using Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.; Clem, Michelle M.

    2009-01-01

    A multiple-point Rayleigh scattering diagnostic is being developed to provide mass flux measurements in gas flows. Spectroscopic Rayleigh scattering is an established flow diagnostic that has the ability to provide simultaneous density, temperature, and velocity measurements. Rayleigh scattered light from a focused 18 Watt continuous-wave laser beam is directly imaged through a solid Fabry-Perot etalon onto a CCD detector which permits spectral analysis of the light. The spatial resolution of the measurements is governed by the locations of interference fringes, which can be changed by altering the etalon characteristics. A prototype system has been used to acquire data in a Mach 0.56 flow to demonstrate feasibility of using this system to provide mass flux measurements. Estimates of measurement uncertainty and recommendations for system improvements are presented

  10. Rayleigh scattering of a Gaussian laser beam from expanding clusters

    SciTech Connect

    Kumar, Manoj; Tripathi, V. K.

    2009-12-15

    Rayleigh scattering of an intense laser with Gaussian temporal and radial profiles from clustered gases is examined. The laser quickly converts the clusters into plasma balls with electron cloud of each ball executing large excursions about the ion sphere. The laser also heats the electrons. As the clusters expand under hydrodynamic pressure, plasma frequency of the cluster electrons omega{sub pe} decreases. The temporal rate of decrease in omega{sub pe} is maximum on laser axis and falls off with r. As the electron density of a cluster approaches plasma resonance, omega{sub pe}=omegasq root(3) (where omega is the frequency of the laser) the oscillatory electron cloud of the cluster produces resonantly enhanced Rayleigh scattering. This resonant enhancement first occurs in clusters on laser axis and afterward in farther clusters. The diffraction divergence of the laser limits the length of the cluster plasma, hence the Rayleigh scattering.

  11. Progress on a Rayleigh Scattering Mass Flux Measurement Technique

    NASA Technical Reports Server (NTRS)

    Mielke-Fagan, Amy F.; Clem, Michelle M.; Elam, Kristie A.; Hirt, Stefanie M.

    2010-01-01

    A Rayleigh scattering diagnostic has been developed to provide mass flux measurements in wind tunnel flows. Spectroscopic molecular Rayleigh scattering is an established flow diagnostic tool that has the ability to provide simultaneous density and velocity measurements in gaseous flows. Rayleigh scattered light from a focused 10 Watt continuous-wave laser beam is collected and fiber-optically transmitted to a solid Fabry-Perot etalon for spectral analysis. The circular interference pattern that contains the spectral information that is needed to determine the flow properties is imaged onto a CCD detector. Baseline measurements of density and velocity in the test section of the 15 cm x 15 cm Supersonic Wind Tunnel at NASA Glenn Research Center are presented as well as velocity measurements within a supersonic combustion ramjet engine isolator model installed in the tunnel test section.

  12. Rayleigh Scattering Diagnostic for Dynamic Measurement of Velocity and Temperature

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Panda, J.

    2001-01-01

    A new technique for measuring dynamic gas velocity and temperature is described. The technique is based on molecular Rayleigh scattering of laser light, so no seeding of the flow is necessary. The Rayleigh scattered light is filtered with a fixed cavity, planar mirror Fabry-Perot interferometer. A minimum number of photodetectors were used in order to allow the high data acquisition rate needed for dynamic measurements. One photomultiplier tube (PMT) was used to measure the total Rayleigh scattering, which is proportional to the gas density. Two additional PMTs were used to detect light that passes through two apertures in a mask located in the interferometer fringe plane. An uncertainty analysis was used to select the optimum aperture parameters and to predict the measurement uncertainty due to photon shot-noise. Results of an experiment to measure the velocity of a subsonic free jet are presented.

  13. Rayleigh scattering in few-mode optical fibers

    PubMed Central

    Wang, Zhen; Wu, Hao; Hu, Xiaolong; Zhao, Ningbo; Mo, Qi; Li, Guifang

    2016-01-01

    The extremely low loss of silica fibers has enabled the telecommunication revolution, but single-mode fiber-optic communication systems have been driven to their capacity limits. As a means to overcome this capacity crunch, space-division multiplexing (SDM) using few-mode fibers (FMF) has been proposed and demonstrated. In single-mode optical fibers, Rayleigh scattering serves as the dominant mechanism for optical loss. However, to date, the role of Rayleigh scattering in FMFs remains elusive. Here we establish and experimentally validate a general model for Rayleigh scattering in FMFs. Rayleigh backscattering not only sets the intrinsic loss limit for FMFs but also provides the theoretical foundation for few-mode optical time-domain reflectometry, which can be used to probe perturbation-induced mode-coupling dynamics in FMFs. We also show that forward inter-modal Rayleigh scattering ultimately sets a fundamental limit on inter-modal-crosstalk for FMFs. Therefore, this work not only has implications specifically for SDM systems but also broadly for few-mode fiber optics and its applications in amplifiers, lasers, and sensors in which inter-modal crosstalk imposes a fundamental performance limitation. PMID:27775003

  14. Rayleigh scattering in few-mode optical fibers.

    PubMed

    Wang, Zhen; Wu, Hao; Hu, Xiaolong; Zhao, Ningbo; Mo, Qi; Li, Guifang

    2016-10-24

    The extremely low loss of silica fibers has enabled the telecommunication revolution, but single-mode fiber-optic communication systems have been driven to their capacity limits. As a means to overcome this capacity crunch, space-division multiplexing (SDM) using few-mode fibers (FMF) has been proposed and demonstrated. In single-mode optical fibers, Rayleigh scattering serves as the dominant mechanism for optical loss. However, to date, the role of Rayleigh scattering in FMFs remains elusive. Here we establish and experimentally validate a general model for Rayleigh scattering in FMFs. Rayleigh backscattering not only sets the intrinsic loss limit for FMFs but also provides the theoretical foundation for few-mode optical time-domain reflectometry, which can be used to probe perturbation-induced mode-coupling dynamics in FMFs. We also show that forward inter-modal Rayleigh scattering ultimately sets a fundamental limit on inter-modal-crosstalk for FMFs. Therefore, this work not only has implications specifically for SDM systems but also broadly for few-mode fiber optics and its applications in amplifiers, lasers, and sensors in which inter-modal crosstalk imposes a fundamental performance limitation.

  15. Rayleigh scattering in few-mode optical fibers

    NASA Astrophysics Data System (ADS)

    Wang, Zhen; Wu, Hao; Hu, Xiaolong; Zhao, Ningbo; Mo, Qi; Li, Guifang

    2016-10-01

    The extremely low loss of silica fibers has enabled the telecommunication revolution, but single-mode fiber-optic communication systems have been driven to their capacity limits. As a means to overcome this capacity crunch, space-division multiplexing (SDM) using few-mode fibers (FMF) has been proposed and demonstrated. In single-mode optical fibers, Rayleigh scattering serves as the dominant mechanism for optical loss. However, to date, the role of Rayleigh scattering in FMFs remains elusive. Here we establish and experimentally validate a general model for Rayleigh scattering in FMFs. Rayleigh backscattering not only sets the intrinsic loss limit for FMFs but also provides the theoretical foundation for few-mode optical time-domain reflectometry, which can be used to probe perturbation-induced mode-coupling dynamics in FMFs. We also show that forward inter-modal Rayleigh scattering ultimately sets a fundamental limit on inter-modal-crosstalk for FMFs. Therefore, this work not only has implications specifically for SDM systems but also broadly for few-mode fiber optics and its applications in amplifiers, lasers, and sensors in which inter-modal crosstalk imposes a fundamental performance limitation.

  16. Control of experimental uncertainties in filtered Rayleigh scattering measurements

    NASA Technical Reports Server (NTRS)

    Forkey, Joseph N.; Finkelstein, N. D.; Lempert, Walter R.; Miles, Richard B.

    1995-01-01

    Filtered Rayleigh Scattering is a technique which allows for measurement of velocity, temperature, and pressure in unseeded flows, spatially resolved in 2-dimensions. We present an overview of the major components of a Filtered Rayleigh Scattering system. In particular, we develop and discuss a detailed theoretical model along with associated model parameters and related uncertainties. Based on this model, we then present experimental results for ambient room air and for a Mach 2 free jet, including spatially resolved measurements of velocity, temperature, and pressure.

  17. Nd:YAG Laser-Based Dual-Line Detection Rayleigh Scattering and Current Efforts on UV, Filtered Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Otugen, M. Volkan; Popovic, Svetozar

    1996-01-01

    Ongoing research in Rayleigh scattering diagnostics for variable density low speed flow applications and for supersonic flow measurements are described. During the past several years, the focus has been on the development and use of a Nd:YAG-based Rayleigh scattering system with improved signal-to-noise characteristics and with applicability to complex, confined flows. This activity serves other research projects in the Aerodynamics Laboratory which require the non-contact, accurate, time-frozen measurement of gas density, pressure, and temperature (each separately), in a fairly wide dynamic range of each parameter. Recently, with the acquisition of a new seed-injected Nd:YAG laser, effort also has been directed to the development of a high-speed velocity probe based on a spectrally resolved Rayleigh scattering technique.

  18. Large-scale inhomogeneity in sapphire test masses revealed by Rayleigh scattering imaging

    NASA Astrophysics Data System (ADS)

    Yan, Zewu; Ju, Li; Eon, François; Gras, Slawomir; Zhao, Chunnong; Jacob, John; Blair, David G.

    2004-03-01

    Rayleigh scattering in test masses can introduce noise and reduce the sensitivity of laser interferometric gravitational wave detectors. In this paper, we present laser Rayleigh scattering imaging as a technique to investigate sapphire test masses. The system provides three-dimensional Rayleigh scattering mapping of entire test masses and quantitative evaluation of the Rayleigh scattering coefficient. Rayleigh scattering mapping of two sapphire samples reveals point defects as well as inhomogeneous structures in the samples. We present results showing significant non-uniform scattering within two 4.5 kg sapphire test masses manufactured by the heat exchanger method.

  19. Rayleigh scattering of a spherical sound wave.

    PubMed

    Godin, Oleg A

    2013-02-01

    Acoustic Green's functions for a homogeneous medium with an embedded spherical obstacle arise in analyses of scattering by objects on or near an interface, radiation by finite sources, sound attenuation in and scattering from clouds of suspended particles, etc. An exact solution of the problem of diffraction of a monochromatic spherical sound wave on a sphere is given by an infinite series involving products of Bessel functions and Legendre polynomials. In this paper, a simple, closed-form solution is obtained for scattering by a sphere with a radius that is small compared to the wavelength. Soft, hard, impedance, and fluid obstacles are considered. The solution is valid for arbitrary positions of the source and receiver relative to the scatterer. Low-frequency scattering is shown to be rather sensitive to boundary conditions on the surface of the obstacle. Low-frequency asymptotics of the scattered acoustic field are extended to transient incident waves. The asymptotic expansions admit an intuitive interpretation in terms of image sources and reduce to classical results in appropriate limiting cases.

  20. In situ characterization of nanoparticles using Rayleigh scattering

    DOE PAGES

    Santra, Biswajit; Shneider, Mikhail N.; Car, Roberto

    2017-01-10

    Here, we report a theoretical analysis showing that Rayleigh scattering could be used to monitor the growth of nanoparticles under arc discharge conditions. We compute the Rayleigh scattering cross sections of the nanoparticles by combining light scattering theory for gas-particle mixtures with calculations of the dynamic electronic polarizability of the nanoparticles. We find that the resolution of the Rayleigh scattering probe is adequate to detect nanoparticles as small as C60 at the expected concentrations of synthesis conditions in the arc periphery. Larger asymmetric nanoparticles would yield brighter signals, making possible to follow the evolution of the growing nanoparticle population frommore » the evolution of the scattered intensity. Observable spectral features include characteristic resonant behaviour, shape-dependent depolarization ratio, and mass-dependent line shape. Direct observation of nanoparticles in the early stages of growth with unobtrusive laser probes should give insight on the particle formation mechanisms and may lead to better-controlled synthesis protocols.« less

  1. Rayleigh scattering and nonlinear inversion of elastic waves

    SciTech Connect

    Gritto, Roland

    1995-12-01

    Rayleigh scattering of elastic waves by an inclusion is investigated and the limitations determined. In the near field of the inhomogeneity, the scattered waves are up to a factor of 300 stronger than in the far field, excluding the application of the far field Rayleigh approximation for this range. The investigation of the relative error as a function of parameter perturbation shows a range of applicability broader than previously assumed, with errors of 37% and 17% for perturbations of -100% and +100%, respectively. The validity range for the Rayleigh limit is controlled by large inequalities, and therefore, the exact limit is determined as a function of various parameter configurations, resulting in surprisingly high values of up to kpR = 0.9. The nonlinear scattering problem can be solved by inverting for equivalent source terms (moments) of the scatterer, before the elastic parameters are determined. The nonlinear dependence between the moments and the elastic parameters reveals a strong asymmetry around the origin, which will produce different results for weak scattering approximations depending on the sign of the anomaly. Numerical modeling of cross hole situations shows that near field terms are important to yield correct estimates of the inhomogeneities in the vicinity of the receivers, while a few well positioned sources and receivers considerably increase the angular coverage, and thus the model resolution of the inversion parameters. The pattern of scattered energy by an inhomogeneity is complicated and varies depending on the object, the wavelength of the incident wave, and the elastic parameters involved. Therefore, it is necessary to investigate the direction of scattered amplitudes to determine the best survey geometry.

  2. Time-Resolved Rayleigh Scattering Measurements in Hot Gas Flows

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.; Sung, Chih-Jen

    2008-01-01

    A molecular Rayleigh scattering technique is developed to measure time-resolved gas velocity, temperature, and density in unseeded gas flows at sampling rates up to 32 kHz. A high power continuous-wave laser beam is focused at a point in an air flow field and Rayleigh scattered light is collected and fiber-optically transmitted to the spectral analysis and detection equipment. The spectrum of the light, which contains information about the temperature and velocity of the flow, is analyzed using a Fabry-Perot interferometer. Photomultipler tubes operated in the photon counting mode allow high frequency sampling of the circular interference pattern to provide time-resolved flow property measurements. Mean and rms velocity and temperature fluctuation measurements in both an electrically-heated jet facility with a 10-mm diameter nozzle and also in a hydrogen-combustor heated jet facility with a 50.8-mm diameter nozzle at NASA Glenn Research Center are presented.

  3. Suppression of Rayleigh-scattering-induced noise in OEOs.

    PubMed

    Okusaga, Olukayode; Cahill, James P; Docherty, Andrew; Menyuk, Curtis R; Zhou, Weimin; Carter, Gary M

    2013-09-23

    Optoelectronic oscillators (OEOs) are hybrid RF-photonic devices that promise to be environmentally robust high-frequency RF sources with very low phase noise. Previously, we showed that Rayleigh-scattering-induced noise in optical fibers coupled with amplitude-to-phase noise conversion in photodetectors and amplifiers leads to fiber-length-dependent noise in OEOs. In this work, we report on two methods for the suppression of this fiber-length-dependent noise: altering the amplitude-dependent phase delay of the OEO loops and suppressing the Rayleigh-scattering-induced noise in optical fibers. We report a 20 dB reduction in the flicker phase noise of a 6 km OEO via these suppression techniques.

  4. Filtered Rayleigh scattering based measurements in compressible mixing layers

    NASA Technical Reports Server (NTRS)

    Elliott, G. S.; Samimy, M.; Arnette, S. A.

    1992-01-01

    Results are presented of experiments in which a Rayleigh-scattering-based technique was used to make quantitative planar measurements in the compressible free shear layers. To this end, the absorption characteristics of the iodine molecular filter were investigated, and initial planar density measurements in M(c) = 0.51 shear layer were performed. The preliminary results presented here demonstrate the validity of the measurement technique.

  5. Experimental study on stimulated Rayleigh scattering in optical fibers.

    PubMed

    Zhu, Tao; Bao, Xiaoyi; Chen, Liang; Liang, Hao; Dong, Yongkang

    2010-10-25

    The linewidth, the threshold, and frequency shift of the stimulated Rayleigh scattering (STRS) in single mode fiber (SMF-28e), large effective area fiber (LEAF) and polarization maintaining fiber (PMF) have been studied using heterodyne detection to separate the Brillouin scattering with a fiber laser for the first time to the best of our knowledge. Experimental results show that the linewidth of STRS and spontaneous Rayleigh scattering are ~9 kHz, ~10 kHz, and ~11 kHz, and ~25 kHz, ~30 kHz, and ~27 kHz for SMF-28e, LEAF and PMF, respectively. The threshold power for STRS for 2 km SMF-28e, 7 km LEAF, and 100 m PMF are 11 dBm, 4.5 dBm and 16.5 dBm, respectively. The measured Rayleigh gain coefficient is a 2 × 10(-13) m/W for SMF-28e. Also, weak frequency shift could be observed when input power is large enough before SBS occurred. Because of the properties of narrower bandwidth and lower threshold power of STRS in fibers, some of applications, such as narrower filter, could be realized.

  6. A Rayleigh-Brillouin scattering spectrometer for ultraviolet wavelengths.

    PubMed

    Gu, Ziyu; Vieitez, M Ofelia; van Duijn, Eric-Jan; Ubachs, Wim

    2012-05-01

    A spectrometer for the measurement of spontaneous Rayleigh-Brillouin (RB) scattering line profiles at ultraviolet wavelengths from gas phase molecules has been developed, employing a high-power frequency-stabilized UV-laser with narrow bandwidth (2 MHz). The UV-light from a frequency-doubled titanium:sapphire laser is further amplified in an enhancement cavity, delivering a 5 W UV-beam propagating through the interaction region inside a scattering cell. The design of the RB-scattering cell allows for measurements at gas pressures in the range 0-4 bars and at stably controlled temperatures from -30 °C to 70 °C. A scannable Fabry-Perot analyzer with instrument resolution of 232 MHz probes the RB profiles. Measurements on N(2) and SF(6) gases demonstrate that the high signal-to-noise ratio is achievable with the instrument at the 1% level at the peak amplitude of the scattering profile.

  7. Rocket plume flowfield characterization using laser Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Zupanc, Frank J.; Weiss, Jonathan M.

    1992-01-01

    A Doppler-resolved laser Rayleigh scattering diagnostic was applied to a 111 N thrust, regenerative and fuel-film cooled, gaseous hydrogen/gaseous oxygen rocket engine. The axial and radial mean gas velocities were measured from the net Doppler shifts observed for two different scattering angles. Translational temperatures and number densities were estimated from the Doppler widths and scattered intensities, respectively, by assuming that water was the dominant scattering species in the exhaust. The experimental results are compared with theoretical predictions from a full Navier-Stokes code (RD/RPLUS) and the JANNAF Two-Dimensional Kinetics (TDK) and Standardized Plume Flowfield (SPF-II) codes. Discrepancies between the measured and predicted axial velocities, temperatures, and number densities are evident. Radial velocity measurements, however, show excellent agreement with predictions. The discrepancies are attributed primarily to inefficient mixing and combustion caused by the injection of excessive oxidizer along one side of the thrust chamber. Thrust and mass flow rate estimates obtained from the Rayleigh measurements show excellent agreement with the globally measured values.

  8. Rocket plume flowfield characterization using laser Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Zupanc, Frank J.; Weiss, Jonathan M.

    1992-07-01

    A Doppler-resolved laser Rayleigh scattering diagnostic was applied to a 111 N thrust, regenerative and fuel-film cooled, gaseous hydrogen/gaseous oxygen rocket engine. The axial and radial mean gas velocities were measured from the net Doppler shifts observed for two different scattering angles. Translational temperatures and number densities were estimated from the Doppler widths and scattered intensities, respectively, by assuming that water was the dominant scattering species in the exhaust. The experimental results are compared with theoretical predictions from a full Navier-Stokes code (RD/RPLUS) and the JANNAF Two-Dimensional Kinetics (TDK) and Standardized Plume Flowfield (SPF-II) codes. Discrepancies between the measured and predicted axial velocities, temperatures, and number densities are evident. Radial velocity measurements, however, show excellent agreement with predictions. The discrepancies are attributed primarily to inefficient mixing and combustion caused by the injection of excessive oxidizer along one side of the thrust chamber. Thrust and mass flow rate estimates obtained from the Rayleigh measurements show excellent agreement with the globally measured values.

  9. Ultraviolet Rayleigh Scatter Imaging for Spatial Temperature Profiles in Atmospheric Microdischarges

    DTIC Science & Technology

    2014-09-01

    laser manufactured by Quantel. This Brilliant laser has a specification output of 330 mJ per pulse at its fundamental 1064 nm, 165 mJ per pulse at...using Rayleigh scattering of a pulsed ultraviolet laser . Scattering intensity images were used to generate a radial profile of translational...agreement with the Rayleigh translational temperature profiles. 15. SUBJECT TERMS ultraviolet laser , Rayleigh scatter microdischarge, translational

  10. Analytical evaluation of atomic form factors: Application to Rayleigh scattering

    SciTech Connect

    Safari, L.; Santos, J. P.; Amaro, P.; Jänkälä, K.; Fratini, F.

    2015-05-15

    Atomic form factors are widely used for the characterization of targets and specimens, from crystallography to biology. By using recent mathematical results, here we derive an analytical expression for the atomic form factor within the independent particle model constructed from nonrelativistic screened hydrogenic wave functions. The range of validity of this analytical expression is checked by comparing the analytically obtained form factors with the ones obtained within the Hartee-Fock method. As an example, we apply our analytical expression for the atomic form factor to evaluate the differential cross section for Rayleigh scattering off neutral atoms.

  11. POLARIZED LIGHT REFLECTED AND TRANSMITTED BY THICK RAYLEIGH SCATTERING ATMOSPHERES

    SciTech Connect

    Natraj, Vijay; Hovenier, J. W.

    2012-03-20

    Accurate values for the intensity and polarization of light reflected and transmitted by optically thick Rayleigh scattering atmospheres with a Lambert surface underneath are presented. A recently reported new method for solving integral equations describing Chandrasekhar's X- and Y-functions is used. The results have been validated using various tests and techniques, including the doubling-adding method, and are accurate to within one unit in the eighth decimal place. Tables are stored electronically and expected to be useful as benchmark results for the (exo)planetary science and astrophysics communities. Asymptotic expressions to obtain Stokes parameters for a thick layer from those of a semi-infinite atmosphere are also provided.

  12. Multiple Point Dynamic Gas Density Measurements Using Molecular Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard; Panda, Jayanta

    1999-01-01

    A nonintrusive technique for measuring dynamic gas density properties is described. Molecular Rayleigh scattering is used to measure the time-history of gas density simultaneously at eight spatial locations at a 50 kHz sampling rate. The data are analyzed using the Welch method of modified periodograms to reduce measurement uncertainty. Cross-correlations, power spectral density functions, cross-spectral density functions, and coherence functions may be obtained from the data. The technique is demonstrated using low speed co-flowing jets with a heated inner jet.

  13. Analytical evaluation of atomic form factors: Application to Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Safari, L.; Santos, J. P.; Amaro, P.; Jänkälä, K.; Fratini, F.

    2015-05-01

    Atomic form factors are widely used for the characterization of targets and specimens, from crystallography to biology. By using recent mathematical results, here we derive an analytical expression for the atomic form factor within the independent particle model constructed from nonrelativistic screened hydrogenic wave functions. The range of validity of this analytical expression is checked by comparing the analytically obtained form factors with the ones obtained within the Hartee-Fock method. As an example, we apply our analytical expression for the atomic form factor to evaluate the differential cross section for Rayleigh scattering off neutral atoms.

  14. Rayleigh scattering in sapphire test mass for laser interferometric gravitational-wave detectors:. II: Rayleigh scattering induced noise in a laser interferometric-wave detector

    NASA Astrophysics Data System (ADS)

    Benabid, F.; Notcutt, M.; Ju, L.; Blair, D. G.

    1999-10-01

    We present the level of noise induced by Rayleigh-scattered light from sapphire test mass, the limit of scattering loss on build-up power inside the interferometer and finally the tolerable absorption loss in order to meet the specification of the interferometer sensitivity. The results show that the Rayleigh scattering induced noise remains below h˜10 -25 Hz -1/2 and a higher tolerance on the absorption level in sapphire substrate compared with silica substrate.

  15. DSMC simulation of Rayleigh-Brillouin scattering in binary mixtures

    NASA Astrophysics Data System (ADS)

    Bruno, Domenico; Frezzotti, Aldo; Ghiroldi, Gian Pietro

    2016-11-01

    Rayleigh-Brillouin scattering spectra (RBS) in dilute gas mixtures have been simulated by the Direct Simulation Monte Carlo method (DSMC). Different noble gas binary mixtures have been considered and the spectra have been simulated adopting the hard sphere collision model. It is suggested that DSMC simulations can be used in the interpretation of light scattering experiments in place of approximate kinetic models. Actually, the former have a firmer physical ground and can be readily extended to treat gas mixtures of arbitrary complexity. The results obtained confirm the capability of DSMC to predict experimental spectra and clears the way towards the simulation of polyatomic gas mixtures of interest for actual application (notably, air) where tractable kinetic model equations are still lacking.

  16. Coherent Rayleigh-Brillouin scattering as a flow diagnostic technique

    SciTech Connect

    Graul, J. S.; Lilly, T. C.

    2014-12-09

    Broadband coherent Rayleigh-Brillouin scattering (CRBS) was used to measure translational gas temperatures for nitrogen at the ambient pressure of 0.8 atm using a purpose-built Fabry-Perot etalon spectrometer. Temperatures derived from the CRBS spectral analysis were compared with experimentally-measured temperatures, and were found to be, on average, within 2% of the experimentally-measured value. Axial flow velocities from a double jet at a pressure ratio of 0.38 were also measured by looking at the Doppler shift of the CRBS line shape. With recent developments in chirped laser technology and the capacity of CRBS to simultaneously provide thermodynamic and bulk flow information, the CRBS line shape acquisition and analysis technique presented here may allow for future time-resolved, characterization of aerospace flows.

  17. Filtered Rayleigh scattering measurements in supersonic/hypersonic facilities

    NASA Technical Reports Server (NTRS)

    Miles, Richard B.; Forkey, Joseph N.; Lempert, Walter R.

    1992-01-01

    Preliminary measurements are presented of flow field properties in Mach 3 and Mach 5 flows using filtered Rayleigh scattering. Filter properties have been characterized by high resolution spectroscopy in order to optimize the selection of laser frequency and filter operating conditions, as well as for the development of an accurate filter modeling program. An optimized filter is used the background suppression feature of this technique to image the boundary layer structure in a Mach 3 high Reynolds number facility and the shock structure in a Mach 5 overexpanded jet. This had been achieved using a visible laser source. By frequency scanning the laser, time-averaged velocity measurements in the Mach 3 and Mach 5 flows are made. Data acquisition at 10 torr and below indicates that this approach can be extrapolated for use in hypersonic flow facilities and is applicable as an in-flight optical air data device for hypersonic vehicles.

  18. Characterization of a Combined CARS and Interferometric Rayleigh Scattering System

    NASA Technical Reports Server (NTRS)

    Tedder, Sarah A.; Bivolaru, Daniel; Danehy, Paul M.; Weikl, M. C.; Beyrau, F.; Seeger, T.; Cutler, Andrew D.

    2007-01-01

    This paper describes the characterization of a combined Coherent anti-Stokes Raman Spectroscopy and Interferometric Rayleigh Scattering (CARS-IRS) system by reporting the accuracy and precision of the measurements of temperature, species mole fraction of N2, O2, and H2, and two-components of velocity. A near-adiabatic H2-air Hencken burner flame was used to provide known properties for measurements made with the system. The measurement system is also demonstrated in a small-scale Mach 1.6 H2-air combustion-heated supersonic jet with a co-flow of H2. The system is found to have a precision that is sufficient to resolve fluctuations of flow properties in the mixing layer of the jet.

  19. Jet Evolution Visualized and Quantified Using Filtered Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Reeder, Mark F.

    1996-01-01

    Filtered Rayleigh scattering was utilized as a flow diagnostic in an investigation of a method for enhancing mixing in supersonic jets. The primary objectives of the study were to visualize the effect of vortex generating tabs on supersonic jets, to exact quantitative data from these planar visualizations, and to detect the presence of secondary flows (i.e., streamwise vorticity) generated by the tabs. An injection seeded frequency-doubled Nd:YAG was the light source and a 14 bit Princeton Instruments iodine charge coupled display (ICCD) camera recorded the image through an iodine cell. The incident wave length of the laser was held constant for each flow case so that the filter absorbed unwanted background light, but permitted part of the thermally broadened Rayleigh scattering light to pas through. The visualizations were performed for axisymmetric jets (D=1.9 cm) operated at perfectly expanded conditions for Mach 1.0, 1.5, and 2.0. All data were recorded for the jet cross section at x/D=3. One hundred instantaneous images were recorded and averaged for each case, with a threshold set to eliminate unavoidable particulate scattering. A key factor in these experiments was that the stagnation air was heated such that the expansion of the flow in the nozzle resulted in the static temperature in the jet being equal to the ambient temperature, assuming isentropic flow. Since the thermodynamic conditions of the flow were approximately the same for each case, increases in the intensity recorded by the ICCD camera could be directly attributed to the Doppler shift, and hence velocity. Visualizations were performed for Mach 1.5 and Mach 2.0 jets with tabs inserted at the nozzle exit. The distortion of the jet was readily apparent and was consistent with Mie scattering-based visualizations. Asymmetry in the intensities of the images indicate the presence of secondary flow patterns which are consistent with the streamwise vortices measured using more traditional diagnostics

  20. Rayleigh Scattering Measurements Using a Tunable Liquid Crystal Fabry-Perot Interferometer

    NASA Technical Reports Server (NTRS)

    Mielke-Fagan, Amy F.; Clem, Michelle M.; Elam, Kristie A.

    2010-01-01

    Spectroscopic Rayleigh scattering is an established flow diagnostic that has the ability to provide simultaneous density, velocity, and temperature measurements. The Fabry-Perot interferometer or etalon is a commonly employed instrument for resolving the spectrum of molecular Rayleigh scattered light for the purpose of evaluating these flow properties. This paper investigates the use of a tunable liquid crystal (LC) Fabry-Perot etalon in Rayleigh scattering experiments at NASA Glenn Research Center. The LC etalon provides a robust interferometry system that can be tuned rapidly by adjusting the voltage applied to the liquid crystal interface. Tuning the interferometer is often necessary to control the physical locations of the concentric interference fringes when Rayleigh light is imaged through the LC etalon. The LC etalon diagnostic system was tested in a 1-cm diameter nozzle flow in two different scattering configurations to evaluate its usefulness for Rayleigh measurements compared to a traditional non-tunable fused silica Fabry-Perot etalon.

  1. Cavity-modified collective Rayleigh scattering of two atoms.

    PubMed

    Reimann, René; Alt, Wolfgang; Kampschulte, Tobias; Macha, Tobias; Ratschbacher, Lothar; Thau, Natalie; Yoon, Seokchan; Meschede, Dieter

    2015-01-16

    We report on the observation of cooperative radiation of exactly two neutral atoms strongly coupled to the single mode field of an optical cavity, which is close to the lossless-cavity limit. Monitoring the cavity output power, we observe constructive and destructive interference of collective Rayleigh scattering for certain relative distances between the two atoms. Because of cavity backaction onto the atoms, the cavity output power for the constructive two-atom case (N=2) is almost equal to the single-emitter case (N=1), which is in contrast to free-space where one would expect an N^{2} scaling of the power. These effects are quantitatively explained by a classical model as well as by a quantum mechanical model based on Dicke states. We extract information on the relative phases of the light fields at the atom positions and employ advanced cooling to reduce the jump rate between the constructive and destructive atom configurations. Thereby we improve the control over the system to a level where the implementation of two-atom entanglement schemes involving optical cavities becomes realistic.

  2. Hyper-Rayleigh scattering of protein-modified gold nanoparticles.

    PubMed

    Zhang, Chun Xiu; Zhang, Yu; Wang, Xin; Tang, Zu Ming; Lu, Zu Hong

    2003-09-01

    The nonlinear optical properties of protein-modified gold nanoparticles has been studied by the hyper-Rayleigh scattering (HRS) technique. HRS signals from the nanoparticles coated with goat-anti-human IgG have been obtained when pumped with a laser pulse with a wavelength of 1064 nm. The HRS signals of gold nanoparticles with IgG were larger than those of bare gold nanoparticles. This can be explained by a noncentrosymmetric effect. It was also found that the HRS signals from the IgG-coated gold nanoparticles could be greatly increased when the antigen was added due to gold nanoparticle aggregation. Our experiment found that the HRS method could produce a measurable signal with 10 microg/ml antigen added, while the colorimetric method using UV spectrum detection required 100 microg/ml of added antigen. The results show that the HRS measurement of immunogold nanoparticles could become a potential immunoassay in determining small levels of antigen in aqueous samples.

  3. Resonance Rayleigh scattering for detection of proteins in HPLC.

    PubMed

    Lu, Xin; Luo, Zhihui; Liu, Chengwei; Zhao, Shulin

    2008-09-01

    An HPLC-resonance Rayleigh scattering (RRS) (HPLC-RRS) detection system is described for separation and detection of proteins. This system is based on the modification of a commercial HPLC instrument involving the addition of a pump and a T-shaped interface, and a common fluorescence detector was used for detection. The detection principle is based on the change of RRS intensity of the ion-association complex formed from biebrich scarlet (BS) and protein. The RRS signal was detected at lambdaex=lambdaem=376 nm. The utility of the presented method was demonstrated by the separation and determination of four proteins involving cytochrome (Cyt-c), lysozyme (Lys), HSA, and gamma-globulin (gamma-Glo). An LOD of 0.2-1.0 microg/mL was reached and a linear range was found between peak area and concentration in the range of 0.20-3.0 microg/mL for Cyt-c, 0.25-2.5 microg/mL for Lys, 1.5-10 microg/mL for HSA, and 2.0-15 microg/mL for gamma-Glo, with linear regression coefficients all above 0.99. The method presented has been applied to determine HSA and gamma-Glo in human serum samples synchronously.

  4. Ultraviolet Molecular Rayleigh Scattering Used to Measure Velocity in High-Speed Flow

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.

    1997-01-01

    Molecular Rayleigh scattering offers a means to measure gas flow parameters including density, temperature, and velocity. No seeding of the flow is necessary. The Rayleigh scattered power is proportional to the gas density, the spectral width is related to the gas temperature, and the shift in the frequency of the spectral peak is proportional to one component of the fluid velocity. Velocity measurements based on Rayleigh scattering are more suitable for high-speed flow, where the bulk fluid velocity is on the order of, or larger than, the molecular thermal velocities. Use of ultraviolet wavelengths for Rayleigh scattering diagnostics is attractive for two reasons. First, the Rayleigh scattering cross section is proportional to the inverse 4th power of the wavelength. And second, the reflectivity of metallic surfaces is generally less than it is at longer wavelengths. This is of particular interest in confined flow situations, such as in small wind tunnels and aircraft engine components, where the stray laser light scattered from the windows and internal surfaces in the test facility limits the application of Rayleigh scattering diagnostics. In this work at the NASA Lewis Research Center, molecular Rayleigh scattering of the 266-nm fourth harmonic of a pulsed, injection seeded Nd:YAG (neodymium:yttriumaluminum- garnet) laser was used to measure velocity in a supersonic free air jet with a 9.3- mm exit diameter. The frequency of the Rayleigh scattered light was analyzed with a planar mirror Fabry-Perot interferometer used in a static imaging mode, with the images recorded on a cooled, high-quantum-efficiency charge-coupled discharge (CCD) camera. In addition, some unshifted light from the same laser pulse was imaged through the interferometer to generate a reference. Data were obtained with single laser pulses at velocities up to Mach 1.3. The measured velocities were in good agreement with velocities calculated from isentropic flow relations. Our conclusion from

  5. Imaging of Passive Scalar Fields by Filtered Rayleigh Scattering

    NASA Astrophysics Data System (ADS)

    Kearney, Sean; Grasser, Thomas; Beresh, Steven; Schefer, Robert

    2002-11-01

    Filtered Rayleigh Scattering (FRS) is a molecular-filter-based, laser-diagnostic approach for multiparameter flowfield imaging that has been gaining popularity over the past 5-10 years [1]. Advantages of FRS for noninvasive gas-phase imaging include: (1) elimination of particle or chemical seeding requirements, (2) increased optical noise rejection allowing imaging close to walls and in "dirty" laboratory environments, (3) imaging of multiple flowfield parameters with a single diagnostic. In this work, the construction and performance of a FRS optical system for passive scalar imaging at Sandia National Laboratories is presented. Data were obtained in an open lab where no special precautions for the elimination of room particulate were made. Results from nonreacting jets and from a premixed flame are shown. Temperature imaging in a nonreacting, steady calibration jet reveals the precision of the time-averaged FRS thermometry results to be ±20 K, or 4of the characteristic temperature difference, while the single-laser-pulse precision is degraded to approximately ±40-50 K. These results are adequate for combustion thermometry purposes. Relative to the jet temperature measurements, species concentration imaging of a buoyant helium jet displays increased signal dynamic range and further improved precision. Reacting flow measurements from the combustion-product region of a methane-air Hencken-type premixed flame are also presented and a comparison of FRS and coherent anti-Stokes Raman scattering (CARS) experiments to calculated adiabatic-equilibrium product temperatures is made which validates the suitability of our FRS instrument for combustion temperature imaging. [1]G.S. Elliott, N. Glumac, and C.D. Carter, Meas. Sci. Tech., 12, 452, 2001.

  6. On the measurement of Rayleigh scattering by gases at 6328A

    NASA Technical Reports Server (NTRS)

    SHARDANAND; Gupta, S. K.

    1973-01-01

    The problem of laboratory measurements of Rayleigh scattering and depolarization ratio for atoms and molecules in the gaseous state is described. It is shown that, if the scattered radiation measurements are made at two angles, the normal depolarization ratio cannot be determined meaningfully. However, from scattering measurements, the Rayleigh scattering cross sections can be determined accurately. The measurements of Raleigh scattering from He, H2, Ar, O2, and N2 for unpolarized radiation at 6328A are reported and compared with similar measurements at 6943 and 1215.7A.

  7. High-speed laser anemometry based on spectrally resolved Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.

    1991-01-01

    Laser anemometry in unseeded flows based on the measurement of the spectrum of Rayleigh scattered laser light is reviewed. The use of molecular scattering avoids the well known problems (particle lag, biasing effects, seed generation, seed injection) of seeded flows. The fundamental limits on velocity measurement accuracy are determined using maximum likelihood methods. Measurement of the Rayleigh spectrum with scanning Fabry-Perot interferometers is analyzed and accuracy limits are established for both single pass and multipass configurations. Multipass configurations have much higher selectivity and are needed for measurements where there is a large amount of excess noise caused by stray laser light. It is shown that Rayleigh scattering is particularly useful for supersonic and hypersonic flows. The results of the analysis are compared with measurements obtained with a Rayleigh scattering diagnostic developed for study of the exhaust plume of a small hydrogen-oxygen rocket, where the velocities are in the range of 1000 to 5000 m/sec.

  8. Investigation of Condensation/Clustering Effects on Rayleigh Scattering Measurements in a Hypersonic Wind Tunnel

    NASA Technical Reports Server (NTRS)

    Tyler, Charles

    1996-01-01

    Rayleigh scattering, a nonintrusive measurement technique for the measurement of density in a hypersonic wind tunnel, is under investigation at Wright Laboratory's Mach 6 wind tunnel. Several adverse effects, i.e., extraneous scatter off walls and windows, hinder Rayleigh scattering measurements. Condensation and clustering of flow constituents also present formidable obstacles. Overcoming some of these difficulties, measurements have been achieved while the Mach 6 test section was pumped down to a vacuum, as well as for actual tunnel operation for various stagnation pressures at fixed stagnation temperatures. Stagnation pressures ranged from 0.69 MPa to 6.9 MPa at fixed stagnation temperatures of 511, 556, and 611 K. Rayleigh scatter results show signal levels much higher than expected for molecular scattering in the wind tunnel. Even with higher than expected signals, scattering measurements have been made in the flowfield of an 8-degree half-angle blunt nose cone with a nose radius of 1.5 cm.

  9. High-spectral-resolution stimulated Rayleigh-Brillouin scattering at 1 microm.

    PubMed

    Faris, G W; Gerken, M; Jirauschek, C; Hogan, D; Chen, Y

    2001-12-01

    We have demonstrated stimulated Rayleigh-Brillouin scattering at a wavelength of 1.064 microm , using an injection-seeded Nd:YAG laser as a pump laser and a tunable diode laser as a probe laser. Spectra with a good signal-to-noise ratio are obtained despite the low probe-beam power and small gain coefficient in the infrared. Stimulated Rayleigh scattering is readily observable in organic and many other liquids because of absorption by the OH and CH overtone or combination bands. The absorption also causes an asymmetry in the stimulated Brillouin peak. A Rayleigh linewidth of 8 MHz is measured with this approach.

  10. Use of two profilers during MCTEX for unambiguous identification of Bragg scattering and Rayleigh scattering

    SciTech Connect

    Gage, K.S.; Williams, C.R.; Ecklund, W.L.; Johnston, P.E.

    1999-11-01

    A 2835-MHz (10.6-cm wavelength) profiler and a 920-MHz (32.6-cm wavelength) profiler were collocated by the NOAA Aeronomy Laboratory at Garden Point, Australia, in the Tiwi Islands during the Maritime Continent Thunderstorm Experiment (MCTEX) field campaign in November and December 1995. The two profilers were directed vertically and observed vertical velocities in the clear atmosphere and hydrometeor fall velocities in deep precipitating cloud systems. In the absence of Rayleigh scatterers, the profilers obtain backscattering from the refractive index irregularities created from atmospheric turbulence acting upon refractive index gradients. This kind of scattering is commonly referred to as Bragg scattering and is only weakly dependent on the radar wavelength provided the radar half-wavelength lies within the inertial subrange of homogeneous, isotropic turbulence. In the presence of hydrometeors the profilers observe Rayleigh backscattering from hydrometeors much as weather radars do and this backscatter is very dependent upon radar wavelength, strongly favoring the shorter wavelength profiler resulting in a 20-dB enhancement of the ability of the 2835-MHz profiler to observe hydrometeors. This paper presents observations of equivalent reflectivity, Doppler velocity, and spectral width made by collocated profilers during MCTEX. Differential reflectivity is used to diagnose the type of echo observed by the profilers in the spectral moment data.

  11. Diode Laser Velocity Measurements by Modulated Filtered Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Mach, J. J.; Varghese, P. L.; Jagodzinski, J. J.

    1999-01-01

    The ability of solid-state lasers to be tuned in operating frequency at MHz rates by input current modulation, while maintaining a relatively narrow line-width, has made them useful for spectroscopic measurements. Their other advantages include low cost, reliability, durability, compact size, and modest power requirements, making them a good choice for a laser source in micro-gravity experiments in drop-towers and in flight. For their size, they are also very bright. In a filtered Rayleigh scattering (FRS) experiment, a diode laser can be used to scan across an atomic or molecular absorption line, generating large changes in transmission at the resonances for very small changes in frequency. The hyperfine structure components of atomic lines of alkali metal vapors are closely spaced and very strong, which makes such atomic filters excellent candidates for sensitive Doppler shift detection and therefore for high-resolution velocimetry. In the work we describe here we use a Rubidium vapor filter, and work with the strong D(sub 2) transitions at 780 nm that are conveniently accessed by near infrared diode lasers. The low power output of infrared laser diodes is their primary drawback relative to other laser systems commonly used for velocimetry. However, the capability to modulate the laser frequency rapidly and continuously helps mitigate this. Using modulation spectroscopy and a heterodyne detection scheme with a lock-in amplifier, one can extract sub-microvolt signals occurring at a specific frequency from a background that is orders of magnitude stronger. The diode laser modulation is simply achieved by adding a small current modulation to the laser bias current. It may also be swept repetitively in wavelength using an additional lower frequency current ramp.

  12. Suppression of Rayleigh scattering noise in sodium laser guide stars by hyperfine depolarization of fluorescence.

    PubMed

    Guillet de Chatellus, Hugues; Moldovan, Ioana; Fesquet, Vincent; Pique, Jean-Paul

    2006-11-27

    We propose what we believe is a novel method for enabling the complete suppression of noise due to Rayleigh scattering in sodium laser guide star systems by means of selective discrimination between Rayleigh and fluorescence signals based on polarization properties. We show that, contrary to the nearly 100% polarized Rayleigh scattering, fluorescence from the D(2) sodium line is strongly depolarized under excitation by a modeless laser. This offers the possibility of completely cancelling the effects of the Rayleigh scattering background while preserving the fluorescence signal to about 40% of its maximal value, leading to an improvement of the signal-to-noise ratio by several orders of magnitude. Both theoretical and experimental data confirm this new proposal.

  13. Individual TiO2 nanocrystals probed by resonant Rayleigh scattering spectroscopy

    NASA Astrophysics Data System (ADS)

    Honda, Mitsuhiro; Saito, Yuika; Kawata, Satoshi

    2014-11-01

    Individual titanium dioxide (TiO2) nanocrystals with bandgaps in the deep ultraviolet (DUV) wavelength range were investigated using resonant Rayleigh scattering spectroscopy. A microscopy system that was switchable from dark-field imaging to scattering spectroscopy was specifically constructed for a broadband UV light source. Weak Rayleigh scattering from a single nanocrystal a few nanometers in size was obtained through the UV excitation resonance and high positional reproducibility of the switching optics. Individual nanocrystals exhibited specific intrinsic bandgaps depending on their size, shape, and crystallinity, greatly affecting their photocatalytic efficiency.

  14. Analysis of the spontaneous Rayleigh-Brillouin scattering spectra of N2

    NASA Astrophysics Data System (ADS)

    Wu, Tao; Xia, Ruxiao; He, Xingdao; Zhang, Xinyi; Yu, Huan

    2016-10-01

    The influence of different pressures, temperatures, scattering angles and incident wavelengths to the relative intensity of the Brillouin peaks to the Rayleigh peak and the Brillouin shift in the spontaneous Rayleigh-Brillouin scattering (SRBS) spectra of N2 is analyzed by using the Tenti S6 model. A system for detecting the SRBS spectra of gas is also introduced in this paper. The SRBS spectra of N2 at different pressures with the incident wavelength of 532nm, the temperature of 300K and the scattering angle of 90° have been measured, the experiment results are well agreed to the simulations.

  15. Mesospheric temperatures from Rayleigh scattering measurements by the WINDII instruments on UARS

    NASA Astrophysics Data System (ADS)

    Evans, W. F. J.; Laframboise, L. R.; Shepherd, G. G.

    1994-09-01

    The WINDII instrument on the UARS satellite has several filter channels. In each of these channels, Rayleigh scattering from the earth's atmosphere is measured in the daytime. The Rayleigh scattering component varies quasi-exponentially with altitude with the scale height of the atmosphere. This data first must be corrected for the relevant baffle scattering component. After several corrections, temperatures from about 75 to 110 km can be measured. The development of the algorithm is discussed and several typical temperature profiles are presented. An analysis of the errors and comparisons with current upper atmosphere models are considered. The presence of nontilucent clouds is indicated in several August profiles in the northern hemisphere.

  16. Gas temperature and density measurements based on spectrally resolved Rayleigh-Brillouin scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Lock, James A.

    1992-01-01

    The use of molecular Rayleigh scattering for measurements of gas density and temperature is evaluated. The technique used is based on the measurement of the spectrum of the scattered light, where both temperature and density are determined from the spectral shape. Planar imaging of Rayleigh scattering from air using a laser light sheet is evaluated for ambient conditions. The Cramer-Rao lower bounds for the shot-noise limited density and temperature measurement uncertainties are calculated for an ideal optical spectrum analyzer and for a planar mirror Fabry-Perot interferometer used in a static, imaging mode. With this technique, a single image of the Rayleigh scattered light can be analyzed to obtain density (or pressure) and temperature. Experimental results are presented for planar measurements taken in a heated air stream.

  17. Demonstration and Analysis of Filtered Rayleigh Scattering Flow Field Diagnostic System

    NASA Technical Reports Server (NTRS)

    Forkey, Joseph N.; Lempert, Walter R.; Miles, Richard B.

    1996-01-01

    Filtered Rayleigh Scattering (FRS) is a diagnostic technique which measures velocity, temperature, and pressure by determining Doppler shift, total intensity, and spectral line shape of laser induced Rayleigh-Brillouin scattering. In the work reported here, this is accomplished by using a narrow line width, injection seeded Nd-YAG laser sheet to induce Rayleigh-Brillouin scattering from a gas flow. This light is passed through an optical notch filter, and transmitted light is imaged onto an intensified charge coupled display (CCD) camera. By monitoring the grayscale value at a particular pixel while the laser frequency is tuned, the convolution between the Rayleigh-Brillouin scattering profile and the filter transmission profile is attained. Since the filter profile can be independently measured, it can be deconvolved from the measuring signal, yielding the Rayleigh-Brillouin scattering profile. From this profile, flow velocity, temperature, and pressure are determined. In this paper the construction and characterization of the optical notch filter and a newly developed frequency apparatus are discussed.

  18. Instantaneous flow measurements in a supersonic wind tunnel using spectrally resolved Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Buggele, Alvin E.; Reeder, Mark F.

    1995-01-01

    Results of a feasibility study to apply laser Rayleigh scattering to non-intrusively measure flow properties in a small supersonic wind tunnel are presented. The technique uses an injection seeded, frequency doubled Nd:YAG laser tuned to an absorption band of iodine. The molecular Rayleigh scattered light is filtered with an iodine cell to block light at the laser frequency. The Doppler-shifted Rayleigh scattered light that passes through the iodine cell is analyzed with a planar mirror Fabry-Perot interferometer used in a static imaging mode. An intensified CCD camera is used to record the images. The images are analyzed at several subregions, where the flow velocity is determined. Each image is obtained with a single laser pulse, giving instantaneous measurements.

  19. Single-Shot Spectrally Resolved UV Rayleigh Scattering Measurements in High Speed Flow

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.

    1996-01-01

    A single-shot UV molecular Rayleigh scattering technique to measure velocity in high speed flow is described. The beam from an injection-seeded, frequency quadrupled Nd:YAG laser (266 nm) is focused to a line in a free air jet with velocities up to Mach 1.3. Rayleigh scattered light is imaged through a planar mirror Fabry-Perot interferometer onto a Charged Coupled Device (CCD) array detector. Some laser light is also simultaneously imaged through the Fabry-Perot to provide a frequency reference. Two velocity measurements are obtained from each image. Multiple-pulse data are also given. The Rayleigh scattering velocity data show good agreement with velocities calculated from isentropic flow relations.

  20. Temperature retrieval error in Rayleigh-Brillouin scattering using Tenti's S6 kinetic model

    NASA Astrophysics Data System (ADS)

    Wu, Lei; Reese, Jason M.; Zhang, Yonghao

    2016-11-01

    The Rayleigh-Brillouin spectrum of light scattered by gas density fluctuations contains information about the gas temperature. This information can be retrieved by comparing experimentally measured spectra with theoretical line shapes determined from the linearized Boltzmann equation. However, the linearized Boltzmann equation is difficult to solve so Tenti's S6 kinetic model has been widely used for several decades because of its simplicity. In this paper, the linearized Boltzmann equation is solved by the efficient fast spectral method, and the temperature retrieval error associated with the Tenti's S6 model is systematically investigated for both spontaneous and coherent Rayleigh-Brillouin scattering, for different gas rarefaction and intermolecular potentials. Our results indicate useful calibrations for laser technologies that use Rayleigh-Brillouin scattering to profile for gas temperatures with high accuracy.

  1. Rayleigh Scattering Diagnostic for Measurement of Temperature and Velocity in Harsh Environments

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Greer, Lawrence C., III

    1998-01-01

    A molecular Rayleigh scattering system for temperature and velocity measurements in unseeded flows is described. The system is capable of making measurements in the harsh environments commonly found in aerospace test facilities, which may have high acoustic sound levels, varying temperatures, and high vibration levels. Light from an argon-ion laser is transmitted via an optical fiber to a remote location where two flow experiments were located. One was a subsonic free air jet; the second was a low-speed heated airjet. Rayleigh scattered light from the probe volume was transmitted through another optical fiber from the remote location to a controlled environment where a Fabry-Perot interferometer and cooled CCD camera were used to analyze the Rayleigh scattered light. Good agreement between the measured velocity and the velocity calculated from isentropic flow relations was demonstrated (less than 5 m/sec). The temperature measurements, however, exhibited systematic errors on the order of 10-15%.

  2. Loss properties due to Rayleigh scattering in different types of fiber.

    PubMed

    Zhi, Wang; Guobin, Ren; Shuqin, Lou; Shuisheng, Jian

    2003-01-13

    The effects of fiber structure on Rayleigh scattering were investigated in detail. Some step-index fibers such as GeO2- and F-doped silica-based fibers and total-internal-reflection photonic crystal fiber are examined. The Rayleigh scattering loss (RSL) depends on the fiber materials and index profiles, and different types of fiber have different dependencies on those parameters because of the different optical power confinement factors in every layer. On the basis of these results, the RSL can be optimized by adjusting the fiber structure or by selecting different materials.

  3. Rayleigh x-ray scattering from many-electron atoms and ions

    NASA Astrophysics Data System (ADS)

    Surzhykov, A.; Yerokhin, V. A.; Stöhlker, Th; Fritzsche, S.

    2015-07-01

    A theoretical analysis is presented for the elastic Rayleigh scattering of x-rays by many-electron atoms and ions. Special emphasis is placed on the angular distribution and linear polarization of the scattered photons for the case when the incident light is completely (linearly) polarized. Based on second-order perturbation theory and the independent particle approximation, we found that the Rayleigh angular distribution is strongly affected by the charge state and shell structure of the target ions or atoms. This effect can be observed experimentally at modern synchrotron facilities and might provide further insight into the structure of heavy atomic systems.

  4. Planar Rayleigh Scattering Results in Helium/Air Mixing Experiments in a Mach 6 Wind Tunnel

    NASA Technical Reports Server (NTRS)

    Shirinzadeh, B.; Balla, R. Jeffrey; Hillard, M. E.; Anders, J. B.; Exton, R. J.; Waitz, I. A.

    1991-01-01

    Planar Rayleigh scattering measurements using an ArF-excimer laser have been performed to investigate helium mixing into air at supersonic speeds. The capability of the Rayleigh scattering technique for flow visualization of a turbulent environment is demonstrated in a large-scale, Mach 6facility. The detection limit obtained with the present setup indicates that planar, quantitative measurements of density can be made over a large cross sectional area (5 cm by 10 cm) of the flow field in the absence of clusters.

  5. Eliminating Rayleigh and Raman Scattering in Three-Dimensional Fluorescence Spectroscopy by Kriging Interpolation

    NASA Astrophysics Data System (ADS)

    Yu, Sh.; Xiao, X.; Xu, G.

    2016-11-01

    In order to effectively eliminate Rayleigh and Raman scattering, a method based on Kriging interpolation is proposed, in which both the distance and the correlation between the scattering region and the nonscattering region are considered. The experimental results show that an unbiased estimation of the scattering region is achieved by this Kriging interpolation. Compared with other interpolation methods that use only the neighboring points, the performance of this method for eliminating the scattering region is much less sensitive to the scattering range that we set.

  6. Multi-Point Interferometric Rayleigh Scattering using Dual-Pass Light Recirculation

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Danehy, Paul M.; Cutler, Andrew D.

    2008-01-01

    This paper describes for the first time an interferometric Rayleigh scattering system using dual-pass light recirculation (IRS-LR) capable of simultaneously measuring at multiple points two orthogonal components of flow velocity in combustion flows using single shot laser probing. An additional optical path containing the interferometer input mirror, a quarter-wave plate, a polarization dependent beam combiner, and a high reflectivity mirror partially recirculates the light that is rejected by the interferometer. Temporally- and spatially-resolved acquisitions of Rayleigh spectra in a large-scale combustion-heated supersonic axi-symmetric jet were performed to demonstrate the technique. Recirculating of Rayleigh scattered light increases the number of photons analyzed by the system up to a factor of 1.8 compared with previous configurations. This is equivalent to performing measurements with less laser energy or performing measurements with the previous system in gas flows at higher temperatures.

  7. Linking Rayleigh-Rice theory with near linear shift invariance in light scattering phenomena

    NASA Astrophysics Data System (ADS)

    Stover, John C.; Schroeder, Sven; Staats, Chris; Lopushenko, Vladimir; Church, Eugene

    2016-09-01

    Understanding topographic scatter has been the subject of many publications. For optically smooth surfaces that scatter only from roughness (and not from contamination, films or bulk defects) the Rayleigh-Rice relationship resulting from a rigorous electromagnetic treatment has been successfully used for over three decades and experimentally proven at wavelengths ranging from the X-Ray to the far infrared (even to radar waves). The "holy grail" of roughness-induced scatter would be a relationship that is not limited to just optically smooth surfaces, but could be used for any surface where the material optical constants and the surface power spectral density function (PSD) are known. Just input these quantities and calculate the BRDF associated with any source incident angle, wavelength and polarization. This is an extremely challenging problem, but that has not stopped a number of attempts. An intuitive requirement on such general relationships is that they must reduce to the simple Rayleigh-Rice formula for sufficiently smooth surfaces. Unfortunately that does not always happen. Because most optically smooth surfaces also scatter from non-topographic features, doubt creeps in about the accuracy of Rayleigh-Rice. This paper investigates these issues and explains some of the confusion generated in recent years. The authors believe there are measurement issues, scatter source issues and rough surface derivation issues, but that Rayleigh- Rice is accurate as formulated and should not be "corrected." Moreover, it will be shown that the empirically observed near shift invariance of surface scatter phenomena is a direct consequence of the Rayleigh-Rice theory.

  8. Direct determination of polymyxin B sulfate using resonance Rayleigh scattering and resonance non-linear scattering methods with hexatungstate.

    PubMed

    Kong, Ling; Liu, Zhongfang; Liu, Shaopu; Wu, Limin; Tian, Fengling

    2014-02-01

    At pH 1.3-1.6, tungstate WO4(2-) , can be converted to hexatungstate W6 O19(2-) , which can react with positively charged polymyxin B sulfate (PMB) to result in enhancement of resonance Rayleigh scattering (RRS) and resonance non-linear scattering, including second order scattering and frequency doubling scattering. Linear relationships can be established between enhanced scattering intensity and PMB concentration. The detection limits (3σ) were 5.5 ng/mL (RRS), 10.1 ng/mL (second order scattering) and 34.6 ng/mL (frequency doubling scattering). The optimum reaction conditions, influencing factors and related analytical properties were tested. The interaction mechanism was investigated via absorption spectrum, circular dichroism spectra and atomic force microscopy imaging. The basis of scattering enhancement is discussed. PMB in eardrops, human serum and urine, were quantified satisfactorily by RRS.

  9. Automatic Rayleigh scattering mapping system for optical quality evaluation of test masses for gravity wave detectors

    NASA Astrophysics Data System (ADS)

    Yan, Zewu; Zhao, Chunnong; Ju, Li; Gras, Slawomir; Baringa, Pablo; Blair, David G.

    2005-01-01

    This article describes an automatic Rayleigh scattering mapping system (ARSMS), which enables quantitative high-resolution three-dimensional mapping of inhomogeneities in optical materials. The ARSMS allows large high-grade test mass samples for gravitational wave detectors to be evaluated to ensure that an adequate low level of scattering is achieved. The ARSMS combines proprietary camera software with data analysis software and control software to achieve fully automatic operation with graphical user interfaces. This article presents the instrument concept and examples of the output. Device mapping in all degrees of freedom is shown to be better than 0.5mm, with scattering sensitivity better than 0.5ppm/cm. This system is able to scan and map the Rayleigh scattering of large samples in both of cylindrical and rectangular samples using cylindrical and Cartesian coordinates.

  10. Study of compressible mixing layers using filtered Rayleigh scattering based visualizations

    NASA Technical Reports Server (NTRS)

    Elliott, Gregory S.; Samimy, MO; Arnette, Stephen A.

    1992-01-01

    Filtered Rayleigh scattering-based flow visualizations of compressible mixing layers are reported. The lower compressibility case (Mc = 0.51) displays well-defined roller-type spanwise structures and streamwise streaks. The structures of the high compressibility case (Mc = 0.86) are more 3D and oblique.

  11. Spatial temperature mapping of an atmospheric microdischarge using ultraviolet Rayleigh scatter imaging

    NASA Astrophysics Data System (ADS)

    Adams, S. F.; Caplinger, J. E.; Sommers, B. S.

    2015-04-01

    Spatially resolved temperature measurements within a microdischarge in atmospheric pressure air have been conducted using Rayleigh scattering of a pulsed ultraviolet laser. Rayleigh scatter images were used to generate highly resolved 1D and 2D profiles of translational temperature, with the analysis based on the ideal gas inverse relationship between temperature and gas density. The technique was shown to be practical to an upper gas temperature limit of approximately 2000 K. Rayleigh scattering results were compared to standard optical emission spectral analyses of {{\\text{N}}2}≤ft({{C}3}{{\\Pi}\\text{u}}\\to {{B}3}{{\\Pi}\\text{g}}\\right) bands, where the calculated rotational temperatures from emission agreed consistently with the peak translational temperatures within the microdischarge measured by Rayleigh laser scatter analyses. The results provide distinctive support of the assumption commonly applied for {{\\text{N}}2} discharges that the {{\\text{N}}2}≤ft({{C}3}{{\\Pi}\\text{u}}\\right) excited state has an identical rotational energy distribution as the {{\\text{N}}2}≤ft({{X}1}{Σ\\text{g}}\\right) ground state. The microdischarge investigated in this study was found to follow another common assumption for non-thermal discharges; that the translation and rotational temperatures are approximately equal to each other and the vibrational temperature is of a much higher value.

  12. High-speed laser anemometry based on spectrally resolved Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, R. G.

    1991-01-01

    Laser anemometry in unseeded flows based on the measurement of the spectrum of Rayleigh scattered laser light is reviewed. The use of molecular scattering avoids the well-known problems (particle lag, biasing effects, seed generation, seed injection) of seeded flows. The fundamental limits on velocity measurement accuracy are determined using maximum likelihood methods. Measurement of the Rayleigh spectrum with scanning Fabry-Perot interferometers is analyzed and accuracy limits are established for both single pass and multi-pass configurations. Multi-pass configurations have much higher selectivity and are needed for measurements where there is a large amount of excess noise caused by stray laser light. It is shown that Rayleigh scattering is particularly useful for supersonic and hypersonic flows. The results of the analysis are compared with measurements obtained with a Rayleigh scattering diagnostic developed for study of the exhaust plume of a small hydrogen-oxygen rocket, where the velocities are in the range 1000 to 5000 m/sec.

  13. Hyper-Rayleigh light scattering from an aqueous suspension of purple membrane.

    PubMed

    Schmidt, P K; Rayfield, G W

    1994-07-01

    Here we report the first observation of hyper-Rayleigh light scattering from bacteriorhodopsin in the form of an aqueous suspension of unoriented purple membranes. A typical purple membrane suspension used in our experiments contains approximately 10(8) randomly oriented purple membranes. Each purple membrane contains approximately 10(5) bacteriorhodopsin molecules in a two-dimensional crystallinearray. Hyper-Rayleigh light scattering is observed when the purple membrane suspension is illuminated with light that has a wavelength of 1064 nm. We propose that the 532-nm scattered light from each of the bacteriorhodopsin molecules in a single purple membrane is coherent, and that the scattered light from different purple membranes is incoherent. This proposal is supported by the following experimental observations: (a) the 532-nm light intensity is proportional to the square of the incident power, (b) the intensity of the 532-nm signal is linearly proportional to the concentration of purple membrane in solution, (c) the scattered 532-nm light is incoherent, (d) the scattered 532-nm light intensity decreases if the size of the purple membranes is reduced while the bacteriorhodopsin concentration is kept constant, and (e) the 532-nm light is due to the retinal chromophore of the bacteriorhodopsin molecule. The ratio of horizontal polarized hyper-Rayleigh scattered light to vertically polarized hyper-Rayleigh scattered light gives the angle (23 ± 4°) of the retinal axis with respect to the plane of the purple membrane. The hyperpolarizability of the bacteriorhodopsin molecule is found to be 5 ± 0.4 × 10(-27) esu.

  14. Superlinear growth of Rayleigh scattering-induced intensity noise in single-mode fibers.

    PubMed

    Cahill, James P; Okusaga, Olukayode; Zhou, Weimin; Menyuk, Curtis R; Carter, Gary M

    2015-03-09

    Rayleigh scattering generates intensity noise close to an optical carrier that propagates in a single-mode optical fiber. This noise degrades the performance of optoelectronic oscillators and RF-photonic links. When using a broad linewidth laser, we previously found that the intensity noise power scales linearly with optical power and fiber length, which is consistent with guided entropy mode Rayleigh scattering (GEMRS), a third order nonlinear scattering process, in the spontaneous limit. In this work, we show that this behavior changes significantly with the use of a narrow linewidth laser. Using a narrow linewidth laser, we measured the bandwidth of the intensity noise plateau to be 10 kHz. We found that the scattered noise power scales superlinearly with fiber length up to lengths of 10 km in the frequency range of 500 Hz to 10 kHz, while it scales linearly in the frequency range of 10 Hz to 100 Hz. These results suggest that the Rayleigh-scattering-induced intensity noise cannot be explained by third-order nonlinear scattering in the spontaneous limit, as previously hypothesized.

  15. Study of Fabry-Perot Etalon Stability and Tuning for Spectroscopic Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Clem, Michelle M.; Mielke-Fagan, Amy F.; Elam, Kristie A.

    2010-01-01

    The Fabry-Perot interferometer is a commonly employed instrument for resolving the spectrum of molecular Rayleigh scattered light for the purpose of evaluating flow properties such as gas velocity and temperature. Rayleigh scattered light from a focused laser beam can be directly imaged through a solid Fabry-Perot etalon onto a CCD detector to provide the spectral content of the scattered light. The spatial resolution of the measurements is governed by the locations of interference fringes. The location of the fringes can be changed by altering the etalon?s physical characteristics, such as thickness and index of refraction. For a fused silica solid etalon the physical properties can be adjusted by changing the etalon temperature; hence changing the order of the interference pattern and the physical fringe locations. Controlling the temperature of the etalon can provide for a slow time-response spatial scanning method for this type of etalon system. A custom designed liquid crystal Fabry-Perot (LCFP) can provide for a fast time-response method of scanning the etalon system. Voltage applied to the liquid crystal interface sets the etalon?s properties allowing Rayleigh measurements to be acquired at varying spatial locations across the image of the laser beam over a very short time period. A standard fused silica etalon and a tunable LCFP etalon are characterized to select the system that is best suited for Rayleigh scattering measurements in subsonic and supersonic flow regimes. A frequency-stabilized laser is used to investigate the apparent frequency stability and temperature sensitivity of the etalon systems. Frequency stability and temperature sensitivity data of the fused silica and LCFP etalon systems are presented in this paper, along with measurements of the LCFP etalon?s tuning capabilities. Rayleigh scattering velocity measurements with both etalon systems are presented, in an effort to determine which etalon is better suited to provide optical flow

  16. Depolarization of laser beam propagating through atmosphere based on multiple Rayleigh scattering model

    NASA Astrophysics Data System (ADS)

    Zhang, Dai; Hao, Shiqi; Wang, Lei; Zhao, Qi

    2016-10-01

    An analytical formula model which is used to describe laser beam's depolarization characteristics is solved based on multiple Rayleigh scattering model. Firstly, by using Stokes vector to characterize intensity and polarization, while at the same time using Mueller matrix and rotation matrix to characterize polarization changing in scattering procedure, a single scattering model is built. Then, a multiple scattering model is built considering the effects of atmospheric absorbing and scattering attenuation. The received light's Stokes vectors through multiple scattering procedure are separately solved. At last, on the basis of multiple scattering vectors, the depolarization characteristics of laser beam propagation through atmosphere are estimated though calculating ratio of depolarization and polarized angle shifting. The numerical analysis based on analytical conclusion of this paper shows that for a horizontal polarized laser beam, its ratio of depolarization is about 1% and polarized angle shifting is about 0.3° when propagates through atmosphere and arrives into the receiver on the ground, and both the above characteristics have only a small change compared with the change of cloud's depth. The findings of these research show that Rayleigh scattering from atmosphere has a weak effect on the laser beam's polarization status. The multiple scattering model and Stokes vector analytical formulas raised in the paper could also be used to study the depolarization characteristics of ellipse polarized laser beam and partially polarized laser beam propagating through atmosphere. The research findings of this paper will have theoretical guiding significances in the domain of laser communication, laser detection and laser imaging.

  17. Rayleigh light scattering properties of atmospheric molecular clusters consisting of sulfuric acid and bases.

    PubMed

    Elm, Jonas; Norman, Patrick; Mikkelsen, Kurt V

    2015-06-28

    The Rayleigh light scattering properties of (H2SO4)a(NH3)b and (H2SO4)a((CH3)2NH)b atmospheric molecular clusters have been investigated using a response theory approach. Using density functional theory the molecular structures and stepwise formation free energies of clusters with a and b up to 4 have been re-investigated. The Rayleigh scattering intensities are calculated from the dipole polarizability tensor α using the CAM-B3LYP functional by applying linear response methods. The intrinsic scattering properties of (H2SO4)a(NH3)b and (H2SO4)a((CH3)2NH)b indicate that amine containing clusters scatter light significantly more efficiently then their ammonia containing counterparts. Using the Atmospheric Cluster Dynamics Code (ACDC) the steady state cluster concentrations are estimated and the effective scattering is calculated. The effective scattering is shown to be highly dependent on the estimated concentrations and indicates that there exist competitive pathways, such as nucleation and coagulation, which influence the cluster distributions. The frequency dependence of the scattering is found to depend on the cluster composition and show increased responses when clusters contain more bases than acid molecules. Based on structures obtained using semi-empirical molecular dynamics simulations the Rayleigh scattering properties of clusters with up to 20 acid-base pairs are evaluated. This study represents the first step towards gaining a fundamental understanding of the scattering properties of small atmospheric clusters in the ambient atmosphere.

  18. Spectrally resolved Rayleigh scattering diagnostic for hydrogen-oxygen rocket plume studies

    NASA Technical Reports Server (NTRS)

    Seasholtz, R. G.; Zupanc, F. J.; Schneider, S. J.

    1991-01-01

    A Rayleigh scattering diagnostic has been developed to measure gas density, temperature, and velocity in the exhaust plume of 100 N thrust class hydrogen-oxygen rockets. The spectrum of argon-ion laser light scattered by the gas molecules in the plume (predominantly water vapor) is measured with a scanning Fabry-Perot interferometer. The gas density is determined from the total scattered power, the gas temperature from the spectral width, and the velocity from the shift in the peak of the spectrum from the frequency of the incident laser light. The diagnostic has been demonstrated in a rocket test cell and a discussion of results is given.

  19. Measuring the scattering mean free path of Rayleigh waves on a volcano from spatial phase decoherence

    NASA Astrophysics Data System (ADS)

    Obermann, Anne; Larose, Eric; Margerin, Ludovic; Rossetto, Vincent

    2014-04-01

    We analyse the statistics of phase fluctuations of seismic signals obtained from a temporary small aperture array deployed on a volcano in the French Auvergne. We demonstrate that the phase field satisfies Circular Gaussian statistics. We then determine the scattering mean free path of Rayleigh waves from the spatial phase decoherence. This phenomenon, observed for diffuse wavefields, is found to yield a good approximation of the scattering mean free path. Contrary to the amplitude, spatial phase decoherence is free from absorption effects and provides direct access to the scattering mean free path.

  20. Ribosome formation from subunits studied by stopped-flow and Rayleigh light scattering

    PubMed Central

    Antoun, Ayman; Pavlov, Michael Y.; Tenson, Tanel

    2004-01-01

    Light scattering and standard stopped-flow techniques were used to monitor rapid association of ribosomal subunits during initiation of eubacterial protein synthesis. The effects of the initiation factors IF1, IF2, IF3 and buffer conditions on subunit association were studied along with the role of GTP in this process. The part of light scattering theory that is essential for kinetic measurements is high-lighted in the main text and a more general treatment of Rayleigh scattering from macromolecules is given in an appendix. PMID:15103398

  1. [Research on detecting concentration of serum protein based on resonance Rayleigh scattering].

    PubMed

    Wang, Gao; Feng, Qiao-Ling; Xue, Zhong-Jin; Li, Yang-Jun; Zhou, Han-Chang

    2013-03-01

    The resonance Rayleigh scattering spectral detection system was designed based on the 2, 9, 16, 23-tetracarboxylate-phthalocyanine zinc and protein system. In the system, excitation light source is 405 nm wide band gap semiconductor lasers, and monochromator is 475 nm narrow-band band-pass filter, and the detector is low-noise and high-gain photoelectric amplifier based on blue-ray enhanced photodiode. Experiment shows that, the solution's strong absorption wavelength is near 420 nm. Under the action of incentive light, resonance Rayleigh scattering is generated at the resonant wavelength, and the scattering intensity is proportional to the protein content. The system uses 2, 9, 16, 23-tetracarboxylate as the spectrum probe to determine the concentration of serum proteins by resonance Rayleigh scattering method. Its linear detection range is 10 - 50 mg.mL-1, and its detection limit is 0. 001 mg.mL-1. The newly developed device for detecting concentration of the serum protein has the advantages of small size, low cost, low power consumption, and being easy to use.

  2. Rayleigh scattering and the internal coupling parameter for arbitrary particle shapes

    NASA Astrophysics Data System (ADS)

    Maughan, Justin B.; Chakrabarti, Amitabha; Sorensen, Christopher M.

    2017-03-01

    A general method for calculating the Rayleigh scattering by a particle of arbitrary shape is introduced. Although analytical solutions for Rayleigh scattering exist for spheres and ellipsoids, analytical solutions for more complicated shapes don't exist. We find that in general the Rayleigh differential cross section goes as k4V2| α (m) | 2 where k = 2 π / λ and λ is the wavelength, V is the volume of the particle and α (m) the average volume polarizability which is dependent on the shape and the complex index of refraction, m. We use existing computational techniques, the discrete dipole approximation (DDA) and the T-matrix method, to calculate the differential scattering cross section divided by k4 and plot it vs V2 to determine | α (m) | 2. Furthermore, we show that this leads to a general description of the internal coupling parameter ρarbitrary‧ = 2 πk V/A | α (m) | where A is the average projected area of the particle in the direction of incident light. It is shown that this general method makes significant changes in the analysis of scattering by particles of any size and shape.

  3. Rayleigh Scattering in the Atmosphere of the Warm Exo-Neptune GJ 3470b

    NASA Astrophysics Data System (ADS)

    Dragomir, Diana; Benneke, Björn; Pearson, Kyle A.; Crossfield, Ian J. M.; Eastman, Jason; Barman, Travis; Biddle, Lauren I.

    2015-12-01

    GJ 3470b is a warm Neptune-size planet transiting an M dwarf star. Like the handful of other small exoplanets for which transmission spectroscopy has been obtained, GJ 3470b exhibits a flat spectrum in the near- and mid-infrared. Recently, a tentative detection of Rayleigh scattering in its atmosphere has been reported. This signal manifests itself as an observed increase of the planetary radius as a function of decreasing wavelength in the visible. We set out to verify this detection and observed several transits of this planet with the LCOGT network and the Kuiper telescope in four different bands (Sloan g, Sloan i, Harris B, and Harris V). Our analysis reveals a strong Rayleigh scattering slope, thus confirming previous results. This makes GJ 3470b the smallest known exoplanet with a detection of Rayleigh scattering. We find that the most plausible scenario is a hydrogen/helium-dominated atmosphere covered by clouds which obscure absorption features in the infrared and hazes which give rise to scattering in the visible. Our results demonstrate the feasibility of exoplanet atmospheric characterization from the ground, even with meter-class telescopes.

  4. RAYLEIGH SCATTERING IN THE ATMOSPHERE OF THE WARM EXO-NEPTUNE GJ 3470B

    SciTech Connect

    Dragomir, Diana; Benneke, Björn; Pearson, Kyle A.; Crossfield, Ian J. M.; Barman, Travis; Eastman, Jason; Biddle, Lauren I.

    2015-12-01

    GJ 3470b is a warm Neptune-size planet transiting an M dwarf star. Like the handful of other small exoplanets for which transmission spectroscopy has been obtained, GJ 3470b exhibits a flat spectrum in the near- and mid-infrared. Recently, a tentative detection of Rayleigh scattering in its atmosphere has been reported. This signal manifests itself as an observed increase of the planetary radius as a function of decreasing wavelength in the visible. We set out to verify this detection and observed several transits of this planet with the LCOGT network and the Kuiper telescope in four different bands (Sloan g, Sloan i, Harris B, and Harris V). Our analysis reveals a strong Rayleigh scattering slope, thus confirming previous results. This makes GJ 3470b the smallest known exoplanet with a detection of Rayleigh scattering. We find that the most plausible scenario is a hydrogen/helium-dominated atmosphere covered by clouds which obscure absorption features in the infrared and hazes which give rise to scattering in the visible. Our results demonstrate the feasibility of exoplanet atmospheric characterization from the ground, even with meter-class telescopes.

  5. Calculations of scattered light from rigid polymers by Shifrin and Rayleigh-Debye approximations.

    PubMed Central

    Bishop, M F

    1989-01-01

    We show that the commonly used Rayleigh-Debye method for calculating light scattering can lead to significant errors when used for describing scattering from dilute solutions of long rigid polymers, errors that can be overcome by use of the easily applied Shifrin approximation. In order to show the extent of the discrepancies between the two methods, we have performed calculations at normal incidence both for polarized and unpolarized incident light with the scattering intensity determined as a function of polarization angle and of scattering angle, assuming that the incident light is in a spectral region where the absorption of hemoglobin is small. When the Shifrin method is used, the calculated intensities using either polarized or unpolarized scattered light give information about the alignment of polymers, a feature that is lost in the Rayleigh-Debye approximation because the effect of the asymmetric shape of the scatterer on the incoming polarized electric field is ignored. Using sickle hemoglobin polymers as an example, we have calculated the intensity of light scattering using both approaches and found that, for totally aligned polymers within parallel planes, the difference can be as large as 25%, when the incident electric field is perpendicular to the polymers, for near forward or near backward scattering (0 degrees or 180 degrees scattering angle), but becomes zero as the scattering angle approaches 90 degrees. For randomly oriented polymers within a plane, or for incident unpolarized light for either totally oriented or randomly oriented polymers, the difference between the two results for near forward or near backward scattering is approximately 15%. PMID:2605302

  6. Dynamics of macroscopic fluctuations in aqueous systems according to Rayleigh scattering data

    NASA Astrophysics Data System (ADS)

    Belovolova, L. V.; Glushkov, M. V.; Timashev, S. F.

    2015-09-01

    The general question of the existence of macrofluctuations of physical characteristics of aqueous systems are discussed. Using the example of analyzing fluctuations in the Rayleigh scattering of natural untreated water, along with catholyte and anolyte obtained in its electrochemical treatment, the possibility of obtaining of quantitative information on the states and dynamics of changes in such systems is shown. Data on the parameters of oscillations in the Rayleigh light scattering of water catholyte and anolyte immediately after electrolysis, and one and two days after its completion, are presented. Calculations are performed using the general phenomenological approach to analyzing chaotic signals (flicker-noise spectroscopy). Quantitative characteristics that reveal substantial differences in the dynamics of macrofluctuations that develop in the catholyte and anolyte of the studied water are presented.

  7. Rayleigh Scattering Diagnostic for Measurement of Velocity and Density Fluctuation Spectra

    NASA Astrophysics Data System (ADS)

    Seasholtz, Richard G.; Panda, Jayanta; Elam, Kristie A.

    2002-04-01

    A new molecular Rayleigh scattering based flow diagnostic is used for the first time to measure the power spectrum of gas density and radial velocity component in the plumes of high speed jets. The technique is based on analyzing the Rayleigh scattered light with a Fabry-Perot interferometer used in the static, imaging mode. The PC based data acquisition system is capable of simultaneous sampling of velocity and density at rates to 100 kHz and data record lengths to 10 million. Velocity and density power spectra and velocity-density cross spectra are presented for a subsonic jet, an underexpanded screeching jet, and for Mach 1.4 and Mach 1.8 supersonic jets. Software and hardware interfaces were developed to allow computer control of all aspects of the experiment and data acquisition.

  8. Rayleigh Scattering Diagnostic for Dynamic Measurement of Velocity Fluctuations in High Speed Jets

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Panda, Jayanta; Elam, Kristie A.

    2001-01-01

    A flow diagnostic technique based on the molecular Rayleigh scattering of laser light is used to obtain dynamic density and velocity data in a high speed flow. The technique is based on analyzing the Rayleigh scattered light with a Fabry-Perot interferometer used in the static, imaging mode. An analysis is presented that established a lower bound for measurement uncertainty of about 20 m/sec for individual velocity measurements obtained in a 100 microsecond time interval. Software and hardware interfaces were developed to allow computer control of all aspects of the experiment and data acquisition. The signals from three photomultiplier tubes were simultaneously recorded using photon counting at a 10 kHz sampling rate and 10 second recording periods. Density and velocity data, including distribution functions and power spectra, taken in a Mach 0.8 free jet, are presented.

  9. Rayleigh Scattering Diagnostic for Measurement of Velocity and Density Fluctuation Spectra

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Panda, Jayanta; Elam, Kristie A.

    2002-01-01

    A new molecular Rayleigh scattering based flow diagnostic is used for the first time to measure the power spectrum of gas density and radial velocity component in the plumes of high speed jets. The technique is based on analyzing the Rayleigh scattered light with a Fabry-Perot interferometer used in the static, imaging mode. The PC based data acquisition system is capable of simultaneous sampling of velocity and density at rates to 100 kHz and data record lengths to 10 million. Velocity and density power spectra and velocity-density cross spectra are presented for a subsonic jet, an underexpanded screeching jet, and for Mach 1.4 and Mach 1.8 supersonic jets. Software and hardware interfaces were developed to allow computer control of all aspects of the experiment and data acquisition.

  10. Rayleigh Scattering Diagnostic for Simultaneous Measurements of Dynamic Density and Velocity

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Panda, J.

    2000-01-01

    A flow diagnostic technique based on the molecular Rayleigh scattering of laser light is used to obtain dynamic density and velocity data in turbulent flows. The technique is based on analyzing the Rayleigh scattered light with a Fabry-Perot interferometer and recording information about the interference pattern with a multiple anode photomultiplier tube (PMT). An artificial neural network is used to process the signals from the PMT to recover the velocity time history, which is then used to calculate the velocity power spectrum. The technique is illustrated using simulated data. The results of an experiment to measure the velocity power spectrum in a low speed (100 rn/sec) flow are also presented.

  11. Reduction of double Rayleigh scattering noise in distributed Raman amplifiers employing higher-order pumping.

    PubMed

    Bolognini, Gabriele; Bononi, Alberto

    2009-04-27

    We present a theoretical study of the performance of distributed Raman amplifiers with higher order pumping schemes, focusing in particular on double Rayleigh scattering (DRS) noise. Results show an unexpected significant DRS noise reduction for pumping order higher than third, allowing for an overall performance improvement of carefully designed distributed amplifiers, ensuring a large optical signal-to-noise ratio improvement together with reduced DRS-induced penalties.

  12. Time Resolved Filtered Rayleigh Scattering Measurement of a Centrifugally Loaded Buoyant Jet

    DTIC Science & Technology

    2011-03-01

    filter along with the transmitted Rayleigh scattering signal [8]. In their study on atomic and molecular notch filters, Miles et al. present...light (broadened and shifted) fell outside the absorption well of the filter while ensuring near total absorbtion of the incident signal itself...Yalin, A.P, Tang, Z, Zaidi, S. H, and Forkey, J.N., “Flow Field Imaging through Sharp-edged Atomic and Molecular ‘Notch’ Filters ”, Measurement

  13. Volumetric imaging of supersonic boundary layers using filtered Rayleigh scattering background suppression

    NASA Technical Reports Server (NTRS)

    Forkey, Joseph N.; Lempert, Walter R.; Bogdonoff, Seymour M.; Miles, Richard B.; Russell, G.

    1995-01-01

    We demonstrate the use of Filtererd Rayleigh Scattering and a 3D reconstruction technique to interrogate the highly three dimensional flow field inside of a supersonic inlet model. A 3 inch by 3 inch by 2.5 inch volume is reconstructed yielding 3D visualizations of the crossing shock waves and of the boundary layer. In this paper we discuss the details of the techniques used, and present the reconstructured 3D images.

  14. Apparatus and Method for Measuring Strain in Optical Fibers using Rayleigh Scatter

    NASA Technical Reports Server (NTRS)

    Froggatt, Mark E. (Inventor); Moore, Jason P. (Inventor)

    2003-01-01

    An apparatus and method for measuring strain in an optical fiber using the spectral shift of Rayleigh scattered light. The interference pattern produced by an air gap reflector and backscattered radiation is measured. Using Fourier Transforms, the spectrum of any section of fiber can be extracted. Cross correlation with an unstrained measurement produces a correlation peak. The location of the correlation peak indicates the strain level in the selected portion of optical fiber.

  15. Application of coherent Rayleigh-Brillouin scattering for in situ nanoparticle and large molecule detection

    NASA Astrophysics Data System (ADS)

    Shneider, M. N.; Gimelshein, S. F.

    2013-04-01

    Feasibility of using coherent Rayleigh-Brillouin scattering for nanoparticle and large molecule diagnostics is assessed analytically and numerically through the solution of the Boltzmann equation. It has been shown that for particles of about 1 nm in diameter dispersed in a buffer gas, concentrations as small as 0.005% may be detected. The approach is expected to provide information on particle concentration with high spatial and temporal resolution.

  16. Retrieval of Temperature From a Multiple Channel Rayleigh-Scatter Lidar Using an Optimal Estimation Method

    NASA Astrophysics Data System (ADS)

    Sica, R. J.; Haefele, A.

    2014-12-01

    The measurement of temperature in the middle atmosphere with Rayleigh-scatter lidars is an important technique for assessing atmospheric change. Current retrieval schemes for these temperature have several shortcoming which can be overcome using an optimal estimation method (OEM). OEMs are applied to the retrieval of temperature from Rayleigh-scatter lidar measurements using both single and multiple channel measurements. Forward models are presented that completely characterize the measurement and allow the simultaneous retrieval of temperature, dead time and background. The method allows a full uncertainty budget to be obtained on a per profile basis that includes, in addition to the statistical uncertainties, the smoothing error and uncertainties due to Rayleigh extinction, ozone absorption, the lidar constant, nonlinearity in the counting system, variation of the Rayleigh-scatter cross section with altitude, pressure, acceleration due to gravity and the variation of mean molecular mass with altitude. The vertical resolution of the temperature profile is found at each height, and a quantitative determination is made of the maximum height to which the retrieval is valid. A single temperature profile can be retrieved from measurements with multiple channels that cover different height ranges, vertical resolutions and even different detection methods. The OEM employed is shown to give robust estimates of temperature consistent with previous methods, while requiring minimal computational time. This demonstrated success of lidar temperature retrievals using an OEM opens new possibilities in atmospheric science for measurement integration between active and passive remote sensing instruments. We are currently working on extending our method to simultaneously retrieve water vapour and temperature using Raman-scatter lidar measurements.

  17. Development of Filtered Rayleigh Scattering for Accurate Measurement of Gas Velocity

    NASA Technical Reports Server (NTRS)

    Miles, Richard B.; Lempert, Walter R.

    1995-01-01

    The overall goals of this research were to develop new diagnostic tools capable of capturing unsteady and/or time-evolving, high-speed flow phenomena. The program centers around the development of Filtered Rayleigh Scattering (FRS) for velocity, temperature, and density measurement, and the construction of narrow linewidth laser sources which will be capable of producing an order MHz repetition rate 'burst' of high power pulses.

  18. Remote-sensing gas measurements with coherent Rayleigh-Brillouin scattering

    DOE PAGES

    Gerakis, A.; Shneider, M. N.; Stratton, B. C.

    2016-07-21

    Here, we measure the coherent Rayleigh-Brillouin scattering (CRBS) signal integral as a function of the recorded gas pressure in He, Co2, SF6, and air, and confirm the already established quadratic dependence of the signal on the gas density. Finally, we propose the use of CRBS as an effective diagnostic for the remote measurement of gas' density (pressure) and temperature, as well as polarizability, for gases of known composition.

  19. Remote-sensing gas measurements with coherent Rayleigh-Brillouin scattering

    SciTech Connect

    Gerakis, A.; Shneider, M. N.; Stratton, B. C.

    2016-07-21

    Here, we measure the coherent Rayleigh-Brillouin scattering (CRBS) signal integral as a function of the recorded gas pressure in He, Co2, SF6, and air, and confirm the already established quadratic dependence of the signal on the gas density. Finally, we propose the use of CRBS as an effective diagnostic for the remote measurement of gas' density (pressure) and temperature, as well as polarizability, for gases of known composition.

  20. Intracavity Rayleigh/Mie Scattering for Multipoint, Two-Component Velocity Measurement

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Danehy, Paul M.; Lee, Joseph W.

    2006-01-01

    A simultaneous multi-point two-component Doppler velocimeter is described. The system uses two optical cavities: a Fabry-Perot etalon and an optical cavity for collecting and re-circulating the Rayleigh/Mie scattered light that is collected from the measurement volume in two parallel, but opposite directions. Single-pulse measurements of two orthogonal components of the velocity vector in a supersonic free jet were performed to demonstrate the technique. The re-circulation of the light rejected by the interferometer input mirror also increased the signal intensity by a factor of 3.5. 2005 Optical Society of America Interferometric Rayleigh scattering has previously been used for single-point velocity measurements in unseeded gas flow. However, this past work has generally been limited to probing with continuous-wave lasers resulting in time-averaged measurements of velocity. Multiple velocity components have been measured simultaneously by separate instruments.1,2 It has also been demonstrated that two orthogonal velocity components can be measured simultaneously at one point using one interferometer by reflecting back the probing laser beam, although this approach results in directional ambiguity of the flow velocity vector.3 This measurement ambiguity was removed by prior knowledge of the approximate magnitude and sign of the velocity components. Furthermore, it was shown that multiple points could be measured simultaneously with a Rayleigh scattering interferometric approach, but only one component of velocity was measured.4 Another method of performing multiple component velocity measurements with Rayleigh scattering uses a pair of cameras to image the flow, one of which views the flow through an iodine gas filter. This iodine-filter technique has the advantage of allowing high-resolution velocity imaging, but it generally has a lower dynamic range.

  1. Remote-sensing gas measurements with coherent Rayleigh-Brillouin scattering

    NASA Astrophysics Data System (ADS)

    Gerakis, A.; Shneider, M. N.; Stratton, B. C.

    2016-07-01

    We measure the coherent Rayleigh-Brillouin scattering (CRBS) signal integral as a function of the recorded gas pressure in He, Co2, SF6, and air, and we confirm the already established quadratic dependence of the signal on the gas density. We propose the use of CRBS as an effective diagnostic for the remote measurement of gas' density (pressure) and temperature, as well as polarizability, for gases of known composition.

  2. Velocity and Temperature Measurement in Supersonic Free Jets Using Spectrally Resolved Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Panda, J.; Seasholtz, R. G.

    2004-01-01

    The flow fields of unheated, supersonic free jets from convergent and convergent-divergent nozzles operating at M = 0.99, 1.4, and 1.6 were measured using spectrally resolved Rayleigh scattering technique. The axial component of velocity and temperature data as well as density data obtained from a previous experiment are presented in a systematic way with the goal of producing a database useful for validating computational fluid dynamics codes. The Rayleigh scattering process from air molecules provides a fundamental means of measuring flow properties in a non-intrusive, particle free manner. In the spectrally resolved application, laser light scattered by the air molecules is collected and analyzed using a Fabry-Perot interferometer (FPI). The difference between the incident laser frequency and the peak of the Rayleigh spectrum provides a measure of gas velocity. The temperature is measured from the spectral broadening caused by the random thermal motion and density is measured from the total light intensity. The present point measurement technique uses a CW laser, a scanning FPI and photon counting electronics. The 1 mm long probe volume is moved from point to point to survey the flow fields. Additional arrangements were made to remove particles from the main as well as the entrained flow and to isolate FPI from the high sound and vibration levels produced by the supersonic jets. In general, velocity is measured within +/- 10 m/s accuracy and temperature within +/- 10 K accuracy.

  3. Spatially-and Temporally-Resolved Multi-Parameter Interferometric Rayleigh Scattering System and Method

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel (Inventor); Cutler, Andrew D. (Inventor); Danehy, Paul M. (Inventor)

    2015-01-01

    A system that simultaneously measures the translational temperature, bulk velocity, and density in gases by collecting, referencing, and analyzing nanosecond time-scale Rayleigh scattered light from molecules is described. A narrow-band pulsed laser source is used to probe two largely separated measurement locations, one of which is used for reference. The elastically scattered photons containing information from both measurement locations are collected at the same time and analyzed spectrally using a planar Fabry-Perot interferometer. A practical means of referencing the measurement of velocity using the laser frequency, and the density and temperature using the information from the reference measurement location maintained at constant properties is provided.

  4. Standoff detection of large organic molecules using Rydberg fingerprint spectroscopy and microwave Rayleigh scattering

    SciTech Connect

    Rudakov, Fedor M; Zhang, Zhili

    2012-01-01

    We present a technique for nonintrusive and standoff detection of large organic molecules using coherent microwave Rayleigh scattering from plasma produced by structure sensitive photoionization through Rydberg states. We test the method on 1,4-diazobicyclooctane. Transitions between the 3s Rydberg state and higher lying Rydberg states are probed using two-color photoionization with 266?nm photons and photons in the range of 460-2400 nm. Photoionization is detected using microwave radiation, which is scattered by the unbounded electrons. Highly resolved Rydberg spectra are acquired in vacuum and in air.

  5. Nonequilibrium fluctuations from a nematic under a thermal gradient and a gravity field*. II. Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Camacho, Jorge F.; Rodríguez, Rosalío F.

    2017-02-01

    The fluctuating hydrodynamic treatment developed in the previous article for a nematic liquid crystal under the influence of a thermal gradient α and a uniform gravity field g, is used to calculate its Rayleigh light scattering spectrum. We find that the dissipative thermal gradient force enhances the Rayleigh-line intensity which varies as k -4 with the fluctuations of the wave number k. The Rayleigh line consists of three central Lorentzians, two of which are determined by the visco-heat modes coupling the entropy and director fluctuations, which is a pure non-equilibrium effect. The third Lorentzian is due only to director fluctuations. We find that the former peaks contain the Rayleigh wings owing to the orientational fluctuations of the aniosotropic molecules. It is also shown that the obtained spectrum reduces to the known equilibrium spectrum of a nematic and to that of a simple fluid. For the particular case in which the decay rates are diffusive, we calculate and plot the amplitudes of non-equilibrium fluctuations of the dynamic structure factor as a function of | α|2/ k 4, and also, the intermediate function in the equilibrium and non-equilibrium states.

  6. Exact Rayleigh scattering calculations for use with the Nimbus-7 Coastal Zone Color Scanner.

    PubMed

    Gordon, H R; Brown, J W; Evans, R H

    1988-03-01

    For improved analysis of Coastal Zone Color Scanner (CZCS) imagery, the radiance reflected from a planeparallel atmosphere and flat sea surface in the absence of aerosols (Rayleigh radiance) has been computed with an exact multiple scattering code, i.e., including polarization. The results indicate that the single scattering approximation normally used to compute this radiance can cause errors of up to 5% for small and moderate solar zenith angles. At large solar zenith angles, such as encountered in the analysis of high-latitude imagery, the errors can become much larger, e.g.,>10% in the blue band. The single scattering error also varies along individual scan lines. Comparison with multiple scattering computations using scalar transfer theory, i.e., ignoring polarization, show that scalar theory can yield errors of approximately the same magnitude as single scattering when compared with exact computations at small to moderate values of the solar zenith angle. The exact computations can be easily incorporated into CZCS processing algorithms, and, for application to future instruments with higher radiometric sensitivity, a scheme is developed with which the effect of variations in the surface pressure could be easily and accurately included in the exact computation of the Rayleigh radiance. Direct application of these computations to CZCS imagery indicates that accurate atmospheric corrections can be made with solar zenith angles at least as large as 65 degrees and probably up to at least 70 degrees with a more sensitive instrument. This suggests that the new Rayleigh radiance algorithm should produce more consistent pigment retrievals, particularly at high latitudes.

  7. Competition between stimulated Brillouin and thermal Rayleigh scattering in Au-nanorods/water system

    NASA Astrophysics Data System (ADS)

    Wu, Haopeng; Shi, Jiulin; Wang, Hongpeng; Qian, Jiacheng; Liu, Juan; He, Xingdao

    2015-04-01

    The use of a simple focused optical cell to present the competition between stimulated Brillouin scattering (SBS) and stimulated thermal Rayleigh scattering (STRS) has been investigated experimentally. An Au-nanorod/water sample as the scattering medium pumped by a pulsed narrow-linewidth second-harmonic Nd:YAG laser with ∼532 nm wavelength, ∼8 ns pulse duration, and 10 Hz repetition rate was used. Experimental results indicate that the absorption coefficient of Au-nanorod/water samples is important for the competition between SBS and STRS. When the absorption coefficient α is smaller than a critical value {{α }cr}, SBS will be dominant during the backward stimulated scattering process. By the same token, when the absorption coefficient α is larger than a critical value {{α }cr}, SBS will be greatly suppressed and STRS will be dominant.

  8. Rayleigh scattering of two x-ray photons by an atom

    NASA Astrophysics Data System (ADS)

    Hopersky, Alexey N.; Nadolinsky, Alexey M.; Novikov, Sergey A.

    2016-05-01

    The process of elastic (Rayleigh) scattering of two x-ray free-electron laser (XFEL) photons by a free He atom is theoretically investigated. We obtain the absolute values and the forms of the triple differential scattering cross section. The main theoretical result is the highest probability of creation of scattered photons with energy ℏ ω±≅ℏ ω ±I1 s (ℏ ω is the energy of the incident XFEL photon, I1 s is the energy of the ionization threshold of the 1 s2 atomic shell). The probability of creation cooled (<ω- ) and hot (>ω+ ) photons is smaller by many orders of magnitude, and is identically zero when the formal (nonphysical) energy of one of the scattered photons is 2 ℏ ω .

  9. Experimental study of unsteady laminar and turbulent flame propagation in an enclosure by Rayleigh scattering

    SciTech Connect

    Tamai, R.; Shepherd, I.G.; Cheng, R.K.

    1992-09-01

    The Rayleigh scattering technique has been used to investigate the flame structure of unsteady propane/air flames propagating under quiescent and turbulent conditions initiated by three ignition methods: (1) conventional spark plug (2) pulse jet combustion (PJC) and (3) Pre-Chamber ignition (PCI). The Rayleigh signal obtained for the laminar cases are all characterized by a sharp transition associated with the large density change which occurs as leading flame front of the expanding flame kernel crosses the measurement point. This indicates that the local flame structures are independent of the ignition source and may be characterized as flamelets. The maximum burning rates deduced from the pressure records show that PJC and PCI increases the burning rate from two to three times above that of conventional spark ignition. The Rayleigh scattering signal obtained for the turbulent cases are also characterized by sharp transition. The wrinkled laminar flamelet model, therefore, provides a valid description of the flame structures for all these unsteady flames. For a given equivalence ratio, the maximum turbulent burning rate deduced for the three turbulent cases with different ignition sources are similar. This suggests that while PJC and PCI enhances burning rate when conditions in the chamber are quiescent, the enhancement is not significant when turbulence fluctuations are present. The PJC and PCI, however, are capable of igniting leaner conditions than the spark plug. This may be due to the injection process which initially disperses ignition sites to a larger volume at a faster rate.

  10. Dynamic Measurement of Temperature, Velocity, and Density in Hot Jets Using Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.

    2009-01-01

    A molecular Rayleigh scattering technique is utilized to measure gas temperature, velocity, and density in unseeded gas flows at sampling rates up to 10 kHz, providing fluctuation information up to 5 kHz based on the Nyquist theorem. A high-power continuous-wave laser beam is focused at a point in an air flow field and Rayleigh scattered light is collected and fiber-optically transmitted to a Fabry-Perot interferometer for spectral analysis. Photomultiplier tubes operated in the photon counting mode allow high-frequency sampling of the total signal level and the circular interference pattern to provide dynamic density, temperature, and velocity measurements. Mean and root mean square velocity, temperature, and density, as well as power spectral density calculations, are presented for measurements in a hydrogen-combustor heated jet facility with a 50.8-mm diameter nozzle at NASA John H. Glenn Research Center at Lewis Field. The Rayleigh measurements are compared with particle image velocimetry data and computational fluid dynamics predictions. This technique is aimed at aeronautics research related to identifying noise sources in free jets, as well as applications in supersonic and hypersonic flows where measurement of flow properties, including mass flux, is required in the presence of shocks and ionization occurrence.

  11. Dynamic Measurement of Temperature, Velocity, and Density in Hot Jets Using Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.

    2008-01-01

    A molecular Rayleigh scattering technique was utilized to measure time-resolved gas temperature, velocity, and density in unseeded gas flows at sampling rates up to 10 kHz. A high power continuous-wave (cw) laser beam was focused at a point in an air flow field and Rayleigh scattered light was collected and fiber-optically transmitted to a Fabry-Perot interferometer for spectral analysis. Photomultipler tubes operated in the photon counting mode allowed high frequency sampling of the total signal level and the circular interference pattern to provide time-resolved density, temperature, and velocity measurements. Mean and rms velocity and temperature, as well as power spectral density calculations, are presented for measurements in a hydrogen-combustor heated jet facility with a 50.8-mm diameter nozzle at the NASA Glenn Research Center (GRC). The Rayleigh measurements are compared with particle image velocimetry data and CFD predictions. This technique is aimed at aeronautics research related to identifying noise sources in free jets, as well as applications in supersonic and hypersonic flows where measurement of flow properties, including mass flux, is required in the presence of shocks and ionization occurrence.

  12. Long-range measurement of Rayleigh scatter signature beyond laser coherence length based on coherent optical frequency domain reflectometry.

    PubMed

    Ohno, Shingo; Iida, Daisuke; Toge, Kunihiro; Manabe, Tetsuya

    2016-08-22

    Long-range C-OFDR measurement of fiber Rayleigh scatter signature is described. The Rayleigh scatter signature, which is an interference pattern of backscatters from the random refractive indices in fibers, is known to be applicable to fiber identification and temperature or strain sensing by measuring its repeatability and its spectral shift. However, these applications have not been realized at ranges beyond the laser coherence length since laser phase noise degrades its repeatability. This paper proposes and demonstrates a method for analyzing the optical power spectrum of local Rayleigh backscatter to overcome the limitation imposed by laser phase noise. The measurable range and spatial performance are also investigated experimentally with respect to the remaining phase noise and noise reduction by signal averaging with the proposed method. The feasibility of Rayleigh scatter signature measurement for long-range applications is confirmed.

  13. Anomalous Rayleigh scattering with dilute concentrations of elements of biological importance

    NASA Astrophysics Data System (ADS)

    Hugtenburg, Richard P.; Bradley, David A.

    2004-01-01

    The anomalous scattering factor (ASF) correction to the relativistic form-factor approximation for Rayleigh scattering is examined in support of its utilization in radiographic imaging. ASF corrected total cross-section data have been generated for a low resolution grid for the Monte Carlo code EGS4 for the biologically important elements, K, Ca, Mn, Fe, Cu and Zn. Points in the fixed energy grid used by EGS4 as well as 8 other points in the vicinity of the K-edge have been chosen to achieve an uncertainty in the ASF component of 20% according to the Thomas-Reiche-Kuhn sum rule and an energy resolution of 20 eV. Such data is useful for analysis of imaging with a quasi-monoenergetic source. Corrections to the sampled distribution of outgoing photons, due to ASF, are given and new total cross-section data including that of the photoelectric effect have been computed using the Slater exchange self-consistent potential with the Latter tail. A measurement of Rayleigh scattering in a dilute aqueous solution of manganese (II) was performed, this system enabling determination of the absolute cross-section, although background subtraction was necessary to remove K β fluorescence and resonant Raman scattering occurring within several 100 eV of the edge. Measurements confirm the presence of below edge bound-bound structure and variation in the structure due to the ionic state that are not currently included in tabulations.

  14. Single-Pulse Multi-Point Multi-Component Interferometric Rayleigh Scattering Velocimeter

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Danehy, Paul M.; Lee, Joseph W.; Gaffney, Richard L., Jr.; Cutler, Andrew D.

    2006-01-01

    A simultaneous multi-point, multi-component velocimeter using interferometric detection of the Doppler shift of Rayleigh, Mie, and Rayleigh-Brillouin scattered light in supersonic flow is described. The system uses up to three sets of collection optics and one beam combiner for the reference laser light to form a single collimated beam. The planar Fabry-Perot interferometer used in the imaging mode for frequency detection preserves the spatial distribution of the signal reasonably well. Single-pulse multi-points measurements of up to two orthogonal and one non-orthogonal components of velocity in a Mach 2 free jet were performed to demonstrate the technique. The average velocity measurements show a close agreement with the CFD calculations using the VULCAN code.

  15. Novel technique for distributed fibre sensing based on coherent Rayleigh scattering measurements of birefringence

    NASA Astrophysics Data System (ADS)

    Lu, Xin; Soto, Marcelo A.; Thévenaz, Luc

    2016-05-01

    A novel distributed fibre sensing technique is described and experimentally validated, based on birefringence measurements using coherent Rayleigh scattering. It natively provides distributed measurements of temperature and strain with more than an order of magnitude higher sensitivity than Brillouin sensing, and requiring access to a single fibre-end. Unlike the traditional Rayleigh-based coherent optical time-domain reflectometry, this new method provides absolute measurements of the measurand and may lead to a robust discrimination between temperature and strain in combination with another technique. Since birefringence is purposely induced in the fibre by design, large degrees of freedom are offered to optimize and scale the sensitivity to a given quantity. The technique has been validated in 2 radically different types of birefringent fibres - elliptical-core and Panda polarization-maintaining fibres - with a good repeatability.

  16. Methods to improve pressure, temperature and velocity accuracies of filtered Rayleigh scattering measurements in gaseous flows

    NASA Astrophysics Data System (ADS)

    Doll, Ulrich; Burow, Eike; Stockhausen, Guido; Willert, Christian

    2016-12-01

    Frequency scanning filtered Rayleigh scattering is able to simultaneously provide time-averaged measurements of pressure, temperature and velocity in gaseous flows. By extending the underlying mathematical model, a robust alternative to existing approaches is introduced. Present and proposed model functions are then characterized during a detailed uncertainty analysis. Deviations between the analytical solution of a jet flow experiment and measured results could be related to laser-induced background radiation as well as the Rayleigh scattering’s spectral distribution. In applying a background correction method and by replacing the standard lineshape model by an empirical formulation, detrimental effects on pressure, temperature and velocity accuracies could be reduced below 15 hPa, 2.5 K and 2.7 m s-1.

  17. Polarization of Rayleigh scattered Lyα in active galactic nuclei

    NASA Astrophysics Data System (ADS)

    Chang, Seok-Jun; Lee, Hee-Won; Yang, Yujin

    2017-02-01

    The unification scheme of active galactic nuclei invokes an optically thick molecular torus component hiding the broad emission line region. Assuming the presence of a thick neutral component in the molecular torus characterized by a H I column density >1022 cm-2, we propose that far-UV radiation around Lyα can be significantly polarized through Rayleigh scattering. Adopting a Monte Carlo technique, we compute polarization of Rayleigh scattered radiation near Lyα in a thick neutral region in the shape of a slab and a cylindrical shell. It is found that radiation near Lyα Rayleigh reflected from a very thick slab can be significantly polarized in a fairly large range of wavelength Δλ ˜ 50 Å exhibiting a flux profile similar to the incident one. Rayleigh transmitted radiation in a slab is characterized by the central dip with a complicated polarization behaviour. The optically thick part near Lyα centre is polarized in the direction perpendicular to the slab normal, which is in contrast to weakly polarized wing parts in the direction parallel to the slab normal. A similar polarization flip phenomenon is also found in the case of a tall cylindrical shell, in which the spatial diffusion along the vertical direction near the inner cylinder wall for core photons leads to a tendency of the electric field aligned to the direction perpendicular to the vertical axis. Observational implications are briefly discussed including spectropolarimetry of the quasar PG 1630+377 by Koratkar et al. in 1990 where Lyα is strongly polarized with no other emission lines polarized.

  18. Fiber optic quench detection via optimized Rayleigh Scattering in high-field YBCO accelerator magnets

    SciTech Connect

    Flanagan, Gene

    2016-02-17

    Yttrium barium copper oxide (YBCO) coated conductors are known for their ability to operate in the superconducting state at relatively high temperatures, even above the boiling point of liquid nitrogen (77 K). When these same conductors are operated at lower temperatures, they are able to operate in much higher magnetic fields than traditional superconductors like NiTi or Nb3Sn. Thus, YBCO superconducting magnets are one of the primary options for generating the high magnetic fields needed for future high energy physics devices. Due to slow quench propagation, quench detection remains one of the primary limitations to YBCO magnets. Fiber optic sensing, based upon Rayleigh scattering, has the potential for spatial resolution approaching the wavelength of light, or very fast temporal resolution at low spatial resolution, and a continuum of combinations in between. This project has studied, theoretically and experimentally, YBCO magnets and Rayleigh scattering quench detection systems to demonstrate feasibility of the systems for YBCO quench protection systems. Under this grant an experimentally validated 3D quench propagation model was used to accurately define the acceptable range of spatial and temporal resolutions for effective quench detection in YBCO magnets and to evaluate present-day and potentially improved YBCO conductors. The data volume and speed requirements for quench detection via Rayleigh scattering required the development of a high performance fiber optic based quench detection/data acquisition system and its integration with an existing voltage tap/thermo-couple based system. In this project, optical fibers are tightly co-wound into YBCO magnet coils, with the fiber on top of the conductor as turn-to-turn insulation. Local changes in the temperature or strain of the conductor are sensed by the optical fiber, which is in close thermal and mechanical contact with the conductor. Intrinsic imperfections in the fiber reflect Rayleigh

  19. Setting up a Rayleigh Scattering Based Flow Measuring System in a Large Nozzle Testing Facility

    NASA Technical Reports Server (NTRS)

    Panda, Jayanta; Gomez, Carlos R.

    2002-01-01

    A molecular Rayleigh scattering based air density measurement system has been built in a large nozzle testing facility at NASA Glenn Research Center. The technique depends on the light scattering by gas molecules present in air; no artificial seeding is required. Light from a single mode, continuous wave laser was transmitted to the nozzle facility by optical fiber, and light scattered by gas molecules, at various points along the laser beam, is collected and measured by photon-counting electronics. By placing the laser beam and collection optics on synchronized traversing units, the point measurement technique is made effective for surveying density variation over a cross-section of the nozzle plume. Various difficulties associated with dust particles, stray light, high noise level and vibration are discussed. Finally, a limited amount of data from an underexpanded jet are presented and compared with expected variations to validate the technique.

  20. Air-mass flux measurement system using Doppler-shifted filtered Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Shirley, John A.; Winter, Michael

    1993-01-01

    An optical system has been investigated to measure mass flux distributions in the inlet of a high speed air-breathing propulsion system. Rayleigh scattered light from air is proportional to the number density of molecules and hence can be used to ascertain the gas density in a calibrated system. Velocity field measurements are achieved by spectrally filtering the elastically-scattered Doppler-shifted light with an absorbing molecular filter. A novel anamorphic optical collection system is used which allows optical rays from different scattering angles, that have different Doppler shifts, to be recorded separately. This is shown to obviate the need to tune the laser through the absorption to determine velocities, while retaining the ability to make spatially-resolved measurements along a line. By properly selecting the laser tuning and filter parameters, simultaneous density measurements can be made. These properties are discussed in the paper and experiments demonstrating the velocimetry capability are described.

  1. Comparison of the GHSSmooth and the Rayleigh-Rice surface scatter theories

    NASA Astrophysics Data System (ADS)

    Harvey, James E.; Pfisterer, Richard N.

    2016-09-01

    The scalar-based GHSSmooth surface scatter theory results in an expression for the BRDF in terms of the surface PSD that is very similar to that provided by the rigorous Rayleigh-Rice (RR) vector perturbation theory. However it contains correction factors for two extreme situations not shared by the RR theory: (i) large incident or scattered angles that result in some portion of the scattered radiance distribution falling outside of the unit circle in direction cosine space, and (ii) the situation where the relevant rms surface roughness, σrel, is less than the total intrinsic rms roughness of the scattering surface. Also, the RR obliquity factor has been discovered to be an approximation of the more general GHSSmooth obliquity factor due to a little-known (or long-forgotten) implicit assumption in the RR theory that the surface autocovariance length is longer than the wavelength of the scattered radiation. This assumption allowed retaining only quadratic terms and lower in the series expansion for the cosine function, and results in reducing the validity of RR predictions for scattering angles greater than 60°. This inaccurate obliquity factor in the RR theory is also the cause of a complementary unrealistic "hook" at the high spatial frequency end of the predicted surface PSD when performing the inverse scattering problem. Furthermore, if we empirically substitute the polarization reflectance, Q, from the RR expression for the scalar reflectance, R, in the GHSSmooth expression, it inherits all of the polarization capabilities of the rigorous RR vector perturbation theory.

  2. Correction of radiation absorption on biological samples using Rayleigh to Compton scattering ratio

    NASA Astrophysics Data System (ADS)

    Pereira, Marcelo O.; Conti, Claudio de Carvalho; dos Anjos, Marcelino J.; Lopes, Ricardo T.

    2012-06-01

    The aim of this work was to develop a method to correct the absorbed radiation (the mass attenuation coefficient curve) in low energy (E < 30 keV) applied to a biological matrix based on the Rayleigh to Compton scattering ratio and the effective atomic number. For calibration, scattering measurements were performed on standard samples of radiation produced by a gamma-ray source of 241Am (59.54 keV) also applied to certified biological samples of milk powder, hay powder and bovine liver (NIST 1557B). In addition, six methods of effective atomic number determination were used as described in literature to determinate the Rayleigh to Compton scattering ratio (R/C), in order to calculate the mass attenuation coefficient. The results obtained by the proposed method were compared with those obtained using the transmission method. The experimental results were in good agreement with transmission values suggesting that the method to correct radiation absorption presented in this paper is adequate for biological samples.

  3. Rayleigh Scattering Diagnostic for Measurement of Temperature, Velocity, and Density Fluctuation Spectra

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.; Sung, Chih-Jen; Panda, Jayanta

    2006-01-01

    A molecular Rayleigh scattering technique is developed to measure dynamic gas temperature, velocity, and density in unseeded turbulent flows at sampling rates up to 10 kHz. A high power CW laser beam is focused at a point in a heated air jet plume and Rayleigh scattered light is collected and spectrally resolved. The spectrum of the light, which contains information about the temperature, velocity, and density of the flow, is analyzed using a Fabry-Perot interferometer. The circular interference fringe pattern is divided into four concentric regions and sampled at 1 and 10 kHz using photon counting electronics. Monitoring the relative change in intensity within each region allows for measurement of gas temperature and velocity. Independently monitoring the total scattered light intensity provides a measure of gas density. Power spectral density calculations of temperature, velocity, and density fluctuations, as well as mean and fluctuating quantities are demonstrated for various radial locations in the jet flow at a fixed axial distance from the jet exit plane. Results are compared with constant current anemometry and pitot probe measurements at the same locations.

  4. Molecular Rayleigh Scattering Diagnostic for Dynamic Temperature, Velocity, and Density Measurements

    NASA Technical Reports Server (NTRS)

    Mielke, Amy R.; Elam, Kristie A.; Sung, Chi-Jen

    2006-01-01

    A molecular Rayleigh scattering technique is developed to measure dynamic gas temperature, velocity, and density in unseeded turbulent flows at sampling rates up to 16 kHz. A high power CW laser beam is focused at a point in an air jet plume and Rayleigh scattered light is collected and spectrally resolved. The spectrum of the light, which contains information about the temperature and velocity of the flow, is analyzed using a Fabry-Perot interferometer. The circular interference fringe pattern is divided into four concentric regions and sampled at 1 and 16 kHz using photon counting electronics. Monitoring the relative change in intensity within each region allows for measurement of gas temperature and velocity. Independently monitoring the total scattered light intensity provides a measure of gas density. A low speed heated jet is used to validate the measurement of temperature fluctuations and an acoustically excited nozzle flow is studied to validate velocity fluctuation measurements. Power spectral density calculations of the property fluctuations, as well as mean and fluctuating quantities are presented. Temperature fluctuation results are compared with constant current anemometry measurements and velocity fluctuation results are compared with constant temperature anemometry measurements at the same locations.

  5. NIR femtosecond laser induced hyper-Rayleigh scattering and luminescence from silver nanoprisms.

    PubMed

    Jain, Beena; Srivastava, Arvind Kumar; Uppal, Abha; Gupta, Pradeep Kumar; Das, Kaustuv

    2010-09-01

    The nonlinear response of silver nanoprisms (edge length 40 +/- 5 nm and thickness 4.5 +/- 0.5 nm) was studied by exciting with NIR femtosecond pulses (780-880 nm). These nanostructures were observed to generate hyper-Rayleigh scattering (HRS) and broadband luminescence. While HRS showed the expected second order power dependence, the luminescence was observed to follow a third order excitation power dependence. Both HRS and luminescence were observed to be dipolar in nature. The first hyperpolarizability of the nanoprisms was found to be an order of magnitude higher than approximately 15 nm sized nanospheres.

  6. Effect of Rayleigh-scattering distributed feedback on multiwavelength Raman fiber laser generation.

    PubMed

    El-Taher, A E; Harper, P; Babin, S A; Churkin, D V; Podivilov, E V; Ania-Castanon, J D; Turitsyn, S K

    2011-01-15

    We experimentally demonstrate a Raman fiber laser based on multiple point-action fiber Bragg grating reflectors and distributed feedback via Rayleigh scattering in an ~22-km-long optical fiber. Twenty-two lasing lines with spacing of ~100 GHz (close to International Telecommunication Union grid) in the C band are generated at the watt level. In contrast to the normal cavity with competition between laser lines, the random distributed feedback cavity exhibits highly stable multiwavelength generation with a power-equalized uniform distribution, which is almost independent on power.

  7. Brillouin-Raman comb fiber laser with cooperative Rayleigh scattering in a linear cavity.

    PubMed

    Zamzuri, A K; Md Ali, M I; Ahmad, A; Mohamad, R; Mahdi, M A

    2006-04-01

    We demonstrate a multiple-wavelength Brillouin comb laser with cooperative Rayleigh scattering that uses Raman amplification in dispersion-compensating fiber. The laser resonator is a linear cavity formed by reflector at each end of the dispersion-compensating fiber to improve the reflectivity of the Brillouin Stokes comb. Multiple Brillouin Stokes generation has been improved in terms of optical signal-to-noise ratio and power-level fluctuation between neighboring channels. Furthermore, the linewidth of the Brillouin Stokes is uniform within the laser output bandwidth.

  8. Time-Average Measurement of Velocity, Density, Temperature, and Turbulence Using Molecular Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Seasholtz, Richard G.; Elam, Krisie A.; Panda, Jayanta

    2004-01-01

    Measurement of time-averaged velocity, density, temperature, and turbulence in gas flows using a nonintrusive, point-wise measurement technique based on molecular Rayleigh scattering is discussed. Subsonic and supersonic flows in a 25.4-mm diameter free jet facility were studied. The developed instrumentation utilizes a Fabry-Perot interferometer to spectrally resolve molecularly scattered light from a laser beam passed through a gas flow. The spectrum of the scattered light contains information about velocity, density, and temperature of the gas. The technique uses a slow scan, low noise 16-bit depth CCD camera to record images of the fringes formed by Rayleigh scattered light passing through the interferometer. A kinetic theory model of the Rayleigh scattered light is used in a nonlinear least squares fitting routine to estimate the unknown parameters from the fringe images. The ability to extract turbulence information from the fringe image data proved to be a challenge since the fringe is broadened by not only turbulence, but also thermal fluctuations and aperture effects from collecting light over a range of scattering angles. Figure 1 illustrates broadening of a Rayleigh spectrum typical of flow conditions observed in this work due to aperture effects and turbulence for a scattering angle, chi(sub s), of 90 degrees, f/3.67 collection optics, mean flow velocity, u(sub k), of 300 m/s, and turbulent velocity fluctuations, sigma (sub uk), of 55 m/s. The greatest difficulty in processing the image data was decoupling the thermal and turbulence broadening in the spectrum. To aid in this endeavor, it was necessary to seed the ambient air with smoke and dust particulates; taking advantage of the turbulence broadening in the Mie scattering component of the spectrum of the collected light (not shown in the figure). The primary jet flow was not seeded due to the difficulty of the task. For measurement points lacking particles, velocity, density, and temperature

  9. A Dual-Line Detection Rayleigh Scattering Diagnostic Technique for the Combustion of Hydrocarbon Fuels and Filtered UV Rayleigh Scattering for Gas Velocity Measurements

    NASA Technical Reports Server (NTRS)

    Otugen, M. Volkan

    1997-01-01

    Non-intrusive techniques for the dynamic measurement of gas flow properties such as density, temperature and velocity, are needed in the research leading to the development of new generation high-speed aircraft. Accurate velocity, temperature and density data obtained in ground testing and in-flight measurements can help understand the flow physics leading to transition and turbulence in supersonic, high-altitude flight. Such non-intrusive measurement techniques can also be used to study combustion processes of hydrocarbon fuels in aircraft engines. Reliable, time and space resolved temperature measurements in various combustor configurations can lead to a better understanding of high temperature chemical reaction dynamics thus leading to improved modeling and better prediction of such flows. In view of this, a research program was initiated at Polytechnic University's Aerodynamics Laboratory with support from NASA Lewis Research Center through grants NAG3-1301 and NAG3-1690. The overall objective of this program has been to develop laser-based, non-contact, space- and time-resolved temperature and velocity measurement techniques. In the initial phase of the program a ND:YAG laser-based dual-line Rayleigh scattering technique was developed and tested for the accurate measurement of gas temperature in the presence of background laser glare. Effort was next directed towards the development of a filtered, spectrally-resolved Rayleigh/Mie scattering technique with the objective of developing an interferometric method for time-frozen velocity measurements in high-speed flows utilizing the uv line of an ND:YAG laser and an appropriate molecular absorption filter. This effort included both a search for an appropriate filter material for the 266 nm laser line and the development and testing of several image processing techniques for the fast processing of Fabry-Perot images for velocity and temperature information. Finally, work was also carried out for the development of

  10. Single-scattering parabolic equation solutions for elastic media propagation, including Rayleigh waves.

    PubMed

    Metzler, Adam M; Siegmann, William L; Collins, Michael D

    2012-02-01

    The parabolic equation method with a single-scattering correction allows for accurate modeling of range-dependent environments in elastic layered media. For problems with large contrasts, accuracy and efficiency are gained by subdividing vertical interfaces into a series of two or more single-scattering problems. This approach generates several computational parameters, such as the number of interface slices, an iteration convergence parameter τ, and the number of iterations n for convergence. Using a narrow-angle approximation, the choices of n=1 and τ=2 give accurate solutions. Analogous results from the narrow-angle approximation extend to environments with larger variations when slices are used as needed at vertical interfaces. The approach is applied to a generic ocean waveguide that includes the generation of a Rayleigh interface wave. Results are presented in both frequency and time domains.

  11. The application of laser Rayleigh scattering to gas density measurements in hypersonic helium flows

    NASA Technical Reports Server (NTRS)

    Hoppe, J. C.; Honaker, W. C.

    1979-01-01

    Measurements of the mean static free-stream gas density have been made in two Langley Research Center helium facilities, the 3-inch leg of the high-Reynolds-number helium complex and the 22-inch hypersonic helium tunnel. Rayleigh scattering of a CW argon ion laser beam at 514.5 nm provided the basic physical mechanism. The behavior of the scattered signal was linear, confirmed by a preliminary laboratory study. That study also revealed the need to introduce baffles to reduce stray light. A relatively simple optical system and associated photon-counting electronics were utilized to obtain data for densities from 10 to the 23rd to 10 to the 25th per cu m. The major purpose, to confirm the applicability of this technique in the hypersonic helium flow, was accomplished.

  12. Direct-View Multi-Point Two-Component Interferometric Rayleigh Scattering Velocimeter

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Danehy, Paul M.; Gaffney, Richard L., Jr.; Cutler, Andrew D.

    2008-01-01

    This paper describes an instantaneous velocity measurement system based on the Doppler shift of elastically scattered laser light from gas molecules (Rayleigh scattering) relative to an incident laser. The system uses a pulsed laser as the light source, direct-viewing optics to collect the scattered light, an interferometer to analyze spectrally the scattered light mixed with the incident laser light, and a CCD camera to capture the resulting interferogram. The system is capable of simultaneous, spatially (approximately 0.2 mm(exp 3)) and temporally (approximately 40 ns) resolved, multiple point measurements of two orthogonal components of flow velocity in the presence of background scattered light, acoustic noise and vibrations, and flow particulates. Measurements in a large-scale axi-symmetric Mach 1.6 H2-air combustion-heated jet running at a flow sensible enthalpy specific to Mach 5.5 hypersonic flight are performed to demonstrate the technique. The measurements are compared with CFD calculations using a finite-volume discretization of the Favre-averaged Navier-Stokes equations (VULCAN code).

  13. Demonstration of Imaging Flow Diagnostics Using Rayleigh Scattering in Langley 0.3-Meter Transonic Cryogenic Tunnel

    NASA Technical Reports Server (NTRS)

    Shirinzadeh, B.; Herring, G. C.; Barros, Toya

    1999-01-01

    The feasibility of using the Rayleigh scattering technique for molecular density imaging of the free-stream flow field in the Langley 0.3-Meter Transonic Cryogenic Tunnel has been experimentally demonstrated. The Rayleigh scattering was viewed with a near-backward geometry with a frequency-doubled output from a diode-pumped CW Nd:YAG laser and an intensified charge-coupled device camera. Measurements performed in the range of free-stream densities from 3 x 10(exp 25) to 24 x 10(exp 25) molecules/cu m indicate that the observed relative Rayleigh signal levels are approximately linear with flow field density. The absolute signal levels agree (within approx. 30 percent) with the expected signal levels computed based on the well-known quantities of flow field density, Rayleigh scattering cross section for N2, solid angle of collection, transmission of the optics, and the independently calibrated camera sensitivity. These results show that the flow field in this facility is primarily molecular (i.e., not contaminated by clusters) and that Rayleigh scattering is a viable technique for quantitative nonintrusive diagnostics in this facility.

  14. Instantaneous 2D Velocity and Temperature Measurements in High Speed Flows Based on Spectrally Resolved Molecular Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.

    1995-01-01

    A Rayleigh scattering diagnostic for high speed flows is described for the simultaneous, instantaneous measurement of gas temperature and velocity at a number (up to about one hundred) of locations in a plane illuminated by an injection-seeded, frequency doubled Nd:YAG laser. Molecular Rayleigh scattered light is collected and passed through a planar mirror Fabry-Perot interferometer. The resulting image is analyzed to determine the gas temperature and bulk velocity at each of the regions. The Cramer Rao lower bound for measurement uncertainty is calculated. Experimental data is presented for a free jet and for preliminary measurements in the Lewis 4 inch by 10 inch supersonic wind tunnel.

  15. Many-electron effects on x-ray Rayleigh scattering by highly charged He-like ions

    NASA Astrophysics Data System (ADS)

    Volotka, A. V.; Yerokhin, V. A.; Surzhykov, A.; Stöhlker, Th.; Fritzsche, S.

    2016-02-01

    The Rayleigh scattering of x rays by many-electron highly charged ions is studied theoretically. The many-electron perturbation theory, based on a rigorous quantum electrodynamics approach, is developed and implemented for the case of the elastic scattering of (high-energetic) photons by heliumlike ions. Using this elaborate approach, we here investigate the many-electron effects beyond the independent-particle approximation (IPA) as conventionally employed for describing the Rayleigh scattering. The total and angle-differential cross sections are evaluated for the x-ray scattering by heliumlike Ni26 +,Xe52 +, and Au77 + ions in their ground state. The obtained results show that, for high-energetic photons, the effects beyond the IPA do not exceed 2% for the scattering by a closed K shell.

  16. Spatially and Temporally-Resolved Multi-Parameter Interferometric Rayleigh Scattering

    NASA Technical Reports Server (NTRS)

    Bivolaru, Daniel; Cutler, Andrew D.; Danehy, Paul M.

    2011-01-01

    A novel approach to simultaneously measure the translational temperature, bulk velocity, and density in gases by collecting, referencing, and analyzing nanosecond time-scale Rayleigh scattered light from molecules is described. A narrow-band pulsed laser source is used to probe two largely separated measurement locations, one of which is used for reference. The elastically scattered photons containing information from both measurement locations are collected at the same time and analyzed spectrally using a planar Fabry - Perot interferometer. A practical means of referencing the measurement of velocity using the laser frequency, and the density and temperature using the information from the reference measurement location maintained at constant properties is described. To demonstrate the technique single-shot spectra of elastic scattered light are obtained in a near zero velocity H2-air Hencken burner flame and simultaneously in an N2-filled gas cell. A simplified Gaussian distribution model to the scattered light spectra is used to obtain the flame properties. Corrections to this model are applied at lower gas temperatures when the simplified Gaussian approximation is no longer suitable. The near-zero measured velocity as a function of the measured flame temperature, and a comparison of the measured flame density and temperature with the perfect gas law are presented.

  17. Interaction of proteins with aluminum(III)-chlorophosphonazo III by resonance Rayleigh scattering method.

    PubMed

    Cui, Zhi-Ping; Liu, Shao-Pu; Liu, Zhong-Fang; Zheng, Hu-Zhi; Hu, Xiao-Li; Xue, Jia-Xing; Tian, Jing

    2014-11-01

    In weak acid medium, aluminum(III) can react with chlorophosphonazo III [CPA(III), H(8)L] to form a 1:1 coordination anion [Al(OH)(H(4)L)](2-). At the same time, proteins such as bovine serum albumin (BSA), lysozyme (Lyso) and human serum albumin (HSA) existed as large cations with positive charges, which further combined with [Al(OH)(H(4)L)](2-) to form a 1:4 chelate. This resulted in significant enhancement of resonance Rayleigh scattering (RRS), second-order scattering (SOS) and frequency doubling scattering (FDS). In this study, we investigated the interaction between [Al(OH)(H(4)L)](2-) and proteins, optimization of the reaction conditions and the spectral characteristics of RRS, SOS and FDS. The maximum RRS wavelengths of different protein systems were located at 357-370 nm. The maximum SOS and FDS wavelengths were located at 546 and 389 nm, respectively. The scattering intensities (ΔI) of the three methods were proportional to the concentration of the proteins, within certain ranges, and the detection limits of the most sensitive RRS method were 2.6-9.3 ng/mL. Moreover, the chelate reaction mechanism or the reasons for the enhancement of RRS were discussed through absorption spectra, fluorescence spectra and circular dichroism (CD) spectra.

  18. Enhancement of Rayleigh scatter in optical fiber by simple UV treatment: an order of magnitude increase in distributed sensing sensitivity

    NASA Astrophysics Data System (ADS)

    Loranger, Sébastien; Parent, François; Lambin-Iezzi, Victor; Kashyap, Raman

    2016-02-01

    Rayleigh scatter in optical fiber communication systems has long been considered a nuisance as a loss mechanism, although applications have used such scatter to probe the fiber for faults and propagation loss using time domain reflectometry (OTDR). It is however only with the development of Frequency domain reflectometry (OFDR) and coherent-phase OTDR that Rayleigh scatter has been probed to its deepest and can now be used to measure strain and temperature along a fiber, leading to the first distributed sensing applications. However, Rayleigh scatter remains very weak giving rise to very small signals which limits the technique for sensing. We show here a new technique to significantly enhance the Rayleigh scatter signal by at least two orders of magnitude, in a standard optical fiber with simple UV exposure of the core. A study of various exposures with different types of fibers has been conducted and a phenomenological description developed. We demonstrate that such an increase in signal can enhance the temperature and strain sensitivity by an order of magnitude for distributed sensing with an OFDR technique. Such improved performance can lead to temperature/strain RMS noise levels of 6 mK and 50 nɛ for 1 cm spatial resolution in UV exposed SMF-28, compared to the typical noise level of 100 mK for the same spatial resolution in the similar unexposed fiber.

  19. A molecular Rayleigh scattering setup to measure density fluctuations in thermal boundary layers

    NASA Astrophysics Data System (ADS)

    Panda, J.

    2016-12-01

    A Rayleigh scattering-based density fluctuation measurement system was set up inside a low-speed wind tunnel of NASA Ames Research Center. The immediate goal was to study the thermal boundary layer on a heated flat plate. A large number of obstacles had to be overcome to set up the system, such as the removal of dust particles using air filters, the use of photoelectron counting electronics to measure low intensity light, an optical layout to minimize stray light contamination, the reduction in tunnel vibration, and an expanded calibration process to relate photoelectron arrival rate to air density close to the plate surface. To measure spectra of turbulent density fluctuations, a two-PMT cross-correlation system was used to minimize the shot noise floor. To validate the Rayleigh measurements, temperature fluctuations spectra were calculated from density spectra and then compared with temperature spectra measured with a cold-wire probe operated in constant current mode. The spectra from the downstream half of the plate were found to be in good agreement with cold-wire probe, whereas spectra from the leading edge differed. Various lessons learnt are discussed. It is believed that the present effort is the first measurement of density fluctuations spectra in a boundary layer flow.

  20. A High Performance Computing approach to model multiple Rayleigh scattering in the Earth atmosphere

    NASA Astrophysics Data System (ADS)

    Franssens, Ghislain; Dekemper, Emmanuel; Mateshivili, Nina; Vanhellemont, filip; fussen, didier; pieroux, didier

    2016-04-01

    The retrieval of atmospheric trace gases and aerosols in the Earth atmosphere from light scattering measurements typically involves an iterative inversion algorithm. A key part of this algorithm is its forward model, which takes care of calculating the amount of light that the remote sensing instrument will see, for any assumed atmosphere composition. The forward model is usually an atmospheric radiative transfer code. It is a serious challenge for a radiative transfer code to be, at the same time, sufficiently accurate and sufficiently fast, so that it can be included in the iterative retrieval loop of an operational service. An accurate code must be able to calculate multiple Rayleigh scattering (important in the UV and/or at lower altitudes) by the air in a spherical atmosphere. This is something that currently only a Monte Carlo algorithm can do. However, any Monte Carlo code is far too slow to be included in the retrieval loop, even if we make use of the currently available HPC power. We report some first results that were obtained by a new solution to this old problem. We first use a HPC cluster to tabulate multiple Rayleigh scattering in a standard Earth atmosphere, using a Monte Carlo code, as function of 6 parameters (albedo, view zenith angle, solar zenith angle, relative azimuth angle, altitude and wavelength). Then, a well chosen empirical function is fitted on the tabulated data. From this function, correction factors are derived and appropriately inserted in a fast single scattering algorithm, which so effectively becomes a multiple scattering algorithm. Since the evaluation of the empirical function is also very fast, we end up with a radiative transfer code that is both accurate and sufficiently fast for operational data production. Our conclusion is that commonly available and affordable HPC systems can still not directly solve the retrieval problem with sufficient accuracy in real time. However, the above described two step approach now becomes

  1. Broadband flat-amplitude multiwavelength Brillouin-Raman fiber laser with spectral reshaping by Rayleigh scattering.

    PubMed

    Wang, Zinan; Wu, Han; Fan, Mengqiu; Li, Yi; Gong, Yuan; Rao, Yunjiang

    2013-12-02

    In this letter, we propose a novel configuration for generating multiwavelength Brillouin-Raman fiber laser (MBRFL). The spectral reshaping effect introduced by Rayleigh scattering in a 50 km single mode fiber unifies the generated Brillouin comb in terms of both power level and linewidth. As a consequence, we are able to obtain a 40 nm flat-amplitude MBRFL with wide bandwidth from 1557 nm to 1597 nm covering >500 Stokes lines. This is, to the best of our knowledge, the widest flat-amplitude bandwidth of MBRFL with uniform Stokes combs using just a single Raman pump laser. The channel-spacing is 0.08 nm and the measured OSNR is higher than 12.5 dB. We also demonstrate that the output spectrum of the MBRFL is nearly unaffected over 14 dB range of Brillouin pumping power.

  2. The development of a tunable, single-frequency ultraviolet laser source for UV filtered Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Finkelstein, N.; Gambogi, J.; Lempert, Walter R.; Miles, Richard B.; Rines, G. A.; Finch, A.; Schwarz, R. A.

    1995-01-01

    We present the development of a flexible, high power, narrow line width, tunable ultraviolet source for diagnostic application. By frequency tripling the output of a pulsed titanium-sapphire laser, we achieve broadly tunable (227-360 nm) ultraviolet light with high quality spatial and spectral resolution. We also present the characterization of a mercury vapor cell which provides a narrow band, sharp edge absorption filter at 253.7 nm. These two components form the basis for the extension of the Filtered Rayleigh Scattering technique into the ultraviolet. The UV-FRS system is comprised of four pieces: a single frequency, cw tunable Ti:Sapphire seeding source; a high-powered pulsed Ti:Sapphire oscillator; a third harmonic generator system; and an atomic mercury vapor filter. In this paper we discuss the development and characterization of each of these elements.

  3. Scattering of Rayleigh-Lamb waves by a surface breaking crack in an elastic plate.

    PubMed

    Flores-López, Miguel A; Gregory, R Douglas

    2006-04-01

    This work studies the problem of scattering of Rayleigh-Lamb waves by a thin surface-breaking crack. The problem is solved by the projection method, which exploits some orthogonality relations deduced from the reciprocal theorem. Numerical results obtained by the projection method are compared with the results obtained using a finite element method reported by other authors for the case of a flat crack, finding good agreement. From the numerical results it is observed that, as the wave number of the incident wave, so for instance, is smaller, the reflected and transmitted energy corresponding to the converted mode, A0 in this case, are almost equal to each other. An explanation for this result is given, based on the asymptotic nature of the modes S0 and A0 for small wave numbers.

  4. [Determination of protein concentration by the enhancement of Rayleigh light scattering of fuchsine acid].

    PubMed

    Zhang, Hong-yi; Liu, Bao-sheng; Zhang, Hong-lei; Zhao, Yong

    2002-12-01

    A new Rayleigh light scattering (RLS) assay is presented in this paper. At the optimum pH = 2.72, the weak RLS of fuchsine acid can be greatly enhanced by the addition of proteins due to the interaction between protein and fuchsine acid. A new quantitative determination method for proteins has been developed. The linear range for human serum albumin is 0-4.0 mg.L-1 with detection limit of 23 micrograms.L-1. Besides high sensitivity, the method is characterized by good reproducibility, rapidity of reaction, good stability and few interfering substances. The determination results of the proteins in human serum and urine samples are very close those obtained using Biuret method, with relative stand deviation of 0.94%-4.93%.

  5. A method of atmospheric density measurements during space shuttle entry using ultraviolet-laser Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Mckenzie, Robert L.

    1988-01-01

    An analytical study and its experimental verification are described which show the performance capabilities and the hardware requirements of a method for measuring atmospheric density along the Space Shuttle flightpath during entry. Using onboard instrumentation, the technique relies on Rayleigh scattering of light from a pulsed ArF excimer laser operating at a wavelength of 193 nm. The method is shown to be capable of providing density measurements with an uncertainty of less than 1 percent and with a spatial resolution along the flightpath of 1 km, over an altitude range from 50 to 90 km. Experimental verification of the signal linearity and the expected signal-to-noise ratios is demonstrated in a simulation facility at conditions that duplicate the signal levels of the flight environment.

  6. A method of atmospheric density measurements during Shuttle entry using UV laser Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Mckenzie, Robert L.

    1987-01-01

    A detailed study is described of the performance capabilities and the hardware requirements for a method in which ambient density is measured along the Space Shuttle flight path using on-board optical instrumentation. The technique relies on Rayleigh scattering of light from a pulsed, ultraviolet, ArF excimer laser operating at a wavelength of 193 nm. The method is shown to be capable of providing direct measurements of ambient density with an uncertainty of less than 1 percent and with a spatial resolution of 1 km, over an altitude range from 50 to 90 km. In addition, extensions of this concept are discussed that allow measurements of the shock wave location and the density profile within the shock layer. Two approaches are identified that appear to be feasible, in which the same laser system is used for the extended measurements as that required for the ambient density measurements.

  7. Molecular Rayleigh Scattering Techniques Developed for Measuring Gas Flow Velocity, Density, Temperature, and Turbulence

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Seasholtz, Richard G.; Elam, Kristie A.; Panda, Jayanta

    2005-01-01

    Nonintrusive optical point-wise measurement techniques utilizing the principles of molecular Rayleigh scattering have been developed at the NASA Glenn Research Center to obtain time-averaged information about gas velocity, density, temperature, and turbulence, or dynamic information about gas velocity and density in unseeded flows. These techniques enable measurements that are necessary for validating computational fluid dynamics (CFD) and computational aeroacoustic (CAA) codes. Dynamic measurements allow the calculation of power spectra for the various flow properties. This type of information is currently being used in jet noise studies, correlating sound pressure fluctuations with velocity and density fluctuations to determine noise sources in jets. These nonintrusive techniques are particularly useful in supersonic flows, where seeding the flow with particles is not an option, and where the environment is too harsh for hot-wire measurements.

  8. A new resonance Rayleigh scattering spectral method for determination of O3 with victoria blue B

    NASA Astrophysics Data System (ADS)

    Wen, Guiqing; Yang, Duo; Jiang, Zhiliang

    2014-01-01

    Ozone (O3) could be absorbed by boric acid-potassium iodide (BKI) absorbent solution to produce tri-iodine ion (I3-) that react with victoria blue B (VBB) to form the associated particle (VBB-I3)n and exhibited a strong resonance Rayleigh scattering (RRS) peak at 722 nm. Under the chosen conditions, the RRS peak intensity was linear with O3 concentration in the range of 0.2-50 μmol/L, with a linear regression equation of ΔI722 = 17.9c - 45.4 and detection limit of 0.057 μmol/L. Accordingly, a simple, rapid and sensitive RRS spectral method was set up for determination of trace O3 in air, with satisfactory results.

  9. Multi-kHz temperature imaging in turbulent non-premixed flames using planar Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Patton, R. A.; Gabet, K. N.; Jiang, N.; Lempert, W. R.; Sutton, J. A.

    2012-08-01

    In this manuscript, we describe the development of two-dimensional, high-repetition-rate (10-kHz) Rayleigh scattering imaging as applied to turbulent combustion environments. In particular, we report what we believe to be the first sets of high-speed planar Rayleigh scattering images in turbulent non-premixed flames, yielding temporally correlated image sequences of the instantaneous temperature field. Sample results are presented for the well-characterized DLR flames A and B (CH4/H2/N2) at Reynolds numbers of 15,200 and 22,800 at various axial positions downstream of the jet exit. The measurements are facilitated by the use of a user-calibrated, intensified, high-resolution CMOS camera in conjunction with a unique high-energy, high-repetition-rate pulse-burst laser system (PBLS) at Ohio State University, which yields output energies up to 200 mJ/pulse at 532 nm with 100-μs laser pulse spacing. The spatial and temporal resolution of the imaging system and acquired images are compared to the finest spatial and temporal scales expected within the turbulent flames. One of the most important features of the PBLS is the ability to readily change the pulse-to-pulse spacing as the required temporal resolution necessitates it. The quality and accuracy of the high-speed temperature imaging results are assessed by comparing derived statistics (mean and standard deviation) to that of previously reported point-based reference data acquired at Sandia National Laboratories and available within the TNF workshop. Good agreement between the two data sets is obtained providing an initial indication of quantitative nature of the planar, kHz-rate temperature imaging results.

  10. POLARIZED PARTIAL FREQUENCY REDISTRIBUTION IN SUBORDINATE LINES. II. SOLUTION OF THE TRANSFER EQUATION WITH RAYLEIGH SCATTERING

    SciTech Connect

    Nagendra, K. N.; Sampoorna, M. E-mail: sampoorna@iiap.res.in

    2012-09-20

    It is quite common in line formation theory to treat scattering in subordinate lines under the assumption of complete frequency redistribution (CRD). The partial frequency redistribution (PRD) in subordinate lines cannot always be approximated by CRD, especially when the polarization state of the line radiation is taken into account. Here we investigate the PRD effects in subordinate lines including scattering polarization. The line formation is described by a polarized non-LTE line transfer equation based on a two-level atom model. We use the recently derived subordinate line redistribution matrix. We devise polarized approximate lambda iteration methods to solve the concerned transfer problem. The linear polarization profiles of subordinate lines formed in non-magnetic (Rayleigh) scattering atmospheres are discussed. We consider one-dimensional isothermal planar model atmospheres. We show that in the polarized line transfer calculations of subordinate lines, PRD plays as important of a role as it does in the case of resonance lines. We also study the effect of collisions on linear polarization profiles of subordinate lines.

  11. Feasibility of Rayleigh Scattering Flow Diagnostics in the National Transonic Facility

    NASA Technical Reports Server (NTRS)

    Herring, Gregory C.; Lee, Joseph W.; Goad, William K.

    2015-01-01

    Laser-based Rayleigh light scattering (RLS) was performed in the National Transonic Facility (NTF) at NASA Langley Research Center. The goal was to determine if the free-stream flow undergoes clustering (early stage of condensation from gas to liquid) or remains in a pure diatomic molecular phase. Data indicate that clusters are not observable down to levels of 10% of the total light scatter for a variety of total pressures at one N2 cryogenic-mode total temperature (Tt = -50 F = 227 K) and one air-mode temperature (Tt = +130 F = 327 K). Thus RLS appears viable as a qualitative or quantitative diagnostic for flow density in NTF in the future. Particles are distinguished from optically unresolvable clusters because they are much larger and individually resolvable in the laser beam image with Mie scattering. The same RLS apparatus was also used, without modification, to visualize naturally occurring particles entrained in the flow for both cryogenic and air-modes. Estimates of the free-stream particle flux are presented, which may be important for interpretation of laminar-to-turbulent boundary-layer transition studies. 1

  12. Interfacing whispering-gallery microresonators and free space light with cavity enhanced Rayleigh scattering

    PubMed Central

    Zhu, Jiangang; Özdemir, Şahin K.; Yilmaz, Huzeyfe; Peng, Bo; Dong, Mark; Tomes, Matthew; Carmon, Tal; Yang, Lan

    2014-01-01

    Whispering gallery mode resonators (WGMRs) take advantage of strong light confinement and long photon lifetime for applications in sensing, optomechanics, microlasers and quantum optics. However, their rotational symmetry and low radiation loss impede energy exchange between WGMs and the surrounding. As a result, free-space coupling of light into and from WGMRs is very challenging. In previous schemes, resonators are intentionally deformed to break circular symmetry to enable free-space coupling of carefully aligned focused light, which comes with bulky size and alignment issues that hinder the realization of compact WGMR applications. Here, we report a new class of nanocouplers based on cavity enhanced Rayleigh scattering from nano-scatterer(s) on resonator surface, and demonstrate whispering gallery microlaser by free-space optical pumping of an Ytterbium doped silica microtoroid via the scatterers. This new scheme will not only expand the range of applications enabled by WGMRs, but also provide a possible route to integrate them into solar powered green photonics. PMID:25227918

  13. Ultrasensitive detection of target analyte-induced aggregation of gold nanoparticles using laser-induced nanoparticle Rayleigh scattering.

    PubMed

    Lin, Jia-Hui; Tseng, Wei-Lung

    2015-01-01

    Detection of salt- and analyte-induced aggregation of gold nanoparticles (AuNPs) mostly relies on costly and bulky analytical instruments. To response this drawback, a portable, miniaturized, sensitive, and cost-effective detection technique is urgently required for rapid field detection and monitoring of target analyte via the use of AuNP-based sensor. This study combined a miniaturized spectrometer with a 532-nm laser to develop a laser-induced Rayleigh scattering technique, allowing the sensitive and selective detection of Rayleigh scattering from the aggregated AuNPs. Three AuNP-based sensing systems, including salt-, thiol- and metal ion-induced aggregation of the AuNPs, were performed to examine the sensitivity of laser-induced Rayleigh scattering technique. Salt-, thiol-, and metal ion-promoted NP aggregation were exemplified by the use of aptamer-adsorbed, fluorosurfactant-stabilized, and gallic acid-capped AuNPs for probing K(+), S-adenosylhomocysteine hydrolase-induced hydrolysis of S-adenosylhomocysteine, and Pb(2+), in sequence. Compared to the reported methods for monitoring the aggregated AuNPs, the proposed system provided distinct advantages of sensitivity. Laser-induced Rayleigh scattering technique was improved to be convenient, cheap, and portable by replacing a diode laser and a miniaturized spectrometer with a laser pointer and a smart-phone. Using this smart-phone-based detection platform, we can determine whether or not the Pb(2+) concentration exceed the maximum allowable level of Pb(2+) in drinking water.

  14. Rayleigh scatter based order of magnitude increase in distributed temperature and strain sensing by simple UV exposure of optical fibre

    PubMed Central

    Loranger, Sébastien; Gagné, Mathieu; Lambin-Iezzi, Victor; Kashyap, Raman

    2015-01-01

    We present a technique to improve signal strength, and therefore sensitivity in distributed temperature and strain sensing (DTSS) using Frequency domain Rayleigh scatter. A simple UV exposure of a hydrogen loaded standard SMF-28 fibre core is shown to enhance the Rayleigh back-scattered light dramatically by ten-fold, independent of the presence of a Bragg grating, and is therefore created by the UV exposure alone. This increase in Rayleigh back-scatter allows an order-of-magnitude increase in temperature and strain resolution for DTSS compared to un-exposed SMF-28 fibre used as a sensing element. This enhancement in sensitivity is effective for cm range or more sensor gauge length, below which is the theoretical cross-correlation limit. The detection of a 20 mK temperature rise with a spatial resolution of 2 cm is demonstrated. This gain in sensitivity for SMF-28 is compared with a high Ge doped photosensitive fibre with a characteristically high NA. For the latter, the UV enhancement is also present although of lower amplitude, and enables an even lower noise level for sensing, due to the fibre’s intrinsically higher Rayleigh scatter signal. PMID:26077365

  15. Filtered Rayleigh scattering diagnostic for multi-parameter thermal-fluids measurements : LDRD final report.

    SciTech Connect

    Beresh, Steven Jay; Grasser, Thomas W.; Kearney, Sean Patrick; Schefer, Robert W.

    2004-01-01

    Simulation-based life-cycle-engineering and the ASCI program have resulted in models of unprecedented size and fidelity. The validation of these models requires high-resolution, multi-parameter diagnostics. Within the thermal-fluids disciplines, the need for detailed, high-fidelity measurements exceeds the limits of current engineering sciences capabilities and severely tests the state of the art. The focus of this LDRD is the development and application of filtered Rayleigh scattering (FRS) for high-resolution, nonintrusive measurement of gas-phase velocity and temperature. With FRS, the flow is laser-illuminated and Rayleigh scattering from naturally occurring sources is detected through a molecular filter. The filtered transmission may be interpreted to yield point or planar measurements of three-component velocities and/or thermodynamic state. Different experimental configurations may be employed to obtain compromises between spatial resolution, time resolution, and the quantity of simultaneously measured flow variables. In this report, we present the results of a three-year LDRD-funded effort to develop FRS combustion thermometry and Aerosciences velocity measurement systems. The working principles and details of our FRS opto-electronic system are presented in detail. For combustion thermometry we present 2-D, spatially correlated FRS results from nonsooting premixed and diffusion flames and from a sooting premixed flame. The FRS-measured temperatures are accurate to within {+-}50 K (3%) in a premixed CH4-air flame and within {+-}100 K for a vortex-strained diluted CH4-air diffusion flame where the FRS technique is severely tested by large variation in scattering cross section. In the diffusion flame work, FRS has been combined with Raman imaging of the CH4 fuel molecule to correct for the local light scattering properties of the combustion gases. To our knowledge, this is the first extension of FRS to nonpremixed combustion and the first use of joint FRS

  16. Highly efficient and two-photon excited stimulated Rayleigh-Bragg scattering in organic solutions

    SciTech Connect

    He, Guang S. Prasad, Paras N.; Kannan, Ramamurthi; Tan, Loon-Seng

    2015-07-21

    The properties of backward stimulated Rayleigh-Bragg scattering (SRBS) in three highly two-photon active AF-chromophores solutions in tetrahydrofuran (THF) have been investigated using 816-nm and 8-ns pump laser beam. The nonlinear reflectivity R, spectral structure, temporal behavior, and phase-conjugation capability of the backward SRBS output have been measured, respectively. Under the same experimental condition, the pump threshold for SRBS in three solution samples can be significantly (∼one order of magnitude) lower than that for stimulated Brillouin scattering (SBS) in the pure solvent (THF). With the optimized concentration value and at a moderate pump energy (∼1.5 mJ) level, the measured nonlinear reflectivity was R ≥ 35% for the 2 cm-long solution sample, while for the SBS from a pure solvent sample of the same length was R ≈ 4.7%. The peculiar features of very low pump threshold, no spectral shift, tolerant pump spectral linewidth requirement (≤1 cm{sup −1}), and phase-conjugation capability are favorable for those nonlinear photonics applications, such as highly efficiency phase-conjugation reflectors for high-brightness laser oscillator/amplifier systems, special imaging through turbid medium, self-adaptive remote optical sensing, as well as for optical rangefinder and lidar systems.

  17. Resonance Rayleigh scattering technique for simple and sensitive analysis of tannic acid with carbon dots

    NASA Astrophysics Data System (ADS)

    Shi, Ying; Yang, Liu; Zhu, Jinghui; Yang, Jidong; Liu, Shaopu; Qiao, Man; Duan, Ruilin; Hu, Xiaoli

    2017-02-01

    Carbon dots (CDs) are raising a substantial amount of attention owing to their many unique and novel physicochemical properties. Herein one-pot synthesized CDs, to the best of our knowledge, were first served as the robust nanoprobe for detection tannic acid (TA) based on resonance Rayleigh scattering technique. The as-prepared CDs can combine with TA via hydrogen bond, resulting in remarkable enhancement of scattering signal with no changes in the fluorescence of CDs. Therefore, a novel protocol for TA determination was established and this strategy allowed quantitative detection of TA in the linear range of 0.2-10.0 μmol L- 1 with an excellent detection limit of 9.0 nmol L- 1. Moreover, the CDs based nanoprobe can be applied to the determination of TA in water sample with satisfactory results. Our study can potentially influence our current views on CDs and particularly impressive and offers new insights into application of CDs beyond the traditional understanding of CDs.

  18. Resonance Rayleigh scattering technique for simple and sensitive analysis of tannic acid with carbon dots.

    PubMed

    Shi, Ying; Yang, Liu; Zhu, Jinghui; Yang, Jidong; Liu, Shaopu; Qiao, Man; Duan, Ruilin; Hu, Xiaoli

    2017-02-15

    Carbon dots (CDs) are raising a substantial amount of attention owing to their many unique and novel physicochemical properties. Herein one-pot synthesized CDs, to the best of our knowledge, were first served as the robust nanoprobe for detection tannic acid (TA) based on resonance Rayleigh scattering technique. The as-prepared CDs can combine with TA via hydrogen bond, resulting in remarkable enhancement of scattering signal with no changes in the fluorescence of CDs. Therefore, a novel protocol for TA determination was established and this strategy allowed quantitative detection of TA in the linear range of 0.2-10.0μmolL(-1) with an excellent detection limit of 9.0nmolL(-1). Moreover, the CDs based nanoprobe can be applied to the determination of TA in water sample with satisfactory results. Our study can potentially influence our current views on CDs and particularly impressive and offers new insights into application of CDs beyond the traditional understanding of CDs.

  19. Rayleigh-Brillouin scattering in SF6 in the kinetic regime

    NASA Astrophysics Data System (ADS)

    Wang, Yuanqing; Yu, Yin; Liang, Kun; Marques, Wilson; van de Water, Willem; Ubachs, Wim

    2017-02-01

    Rayleigh-Brillouin spectral profiles are measured with a laser-based scatterometry setup for a 90° scattering angle at a high signal-to-noise ratio (r.m.s. noise below 0.15% w.r.t. peak intensity) in sulfur-hexafluoride gas for pressures in the range 0.2-5 bar and for a wavelength of λ = 403.0 nm. The high quality data are compared to a number of light scattering models in order to address the effects of rotational and vibrational relaxation. While the vibrational relaxation rate is so slow that vibration degrees of freedom remain frozen, rotations relax on time scales comparable to those of the density fluctuations. Therefore, the heat capacity, the thermal conductivity and the bulk viscosity are all frequency-dependent transport coefficients. This is relevant for the Tenti model that depends on the values chosen for these transport coefficients. This is not the case for the other two models considered: a kinetic model based on rough-sphere interactions, and a model based on fluctuating hydrodynamics. The deviations with the experiment are similar between the three different models, except for the hydrodynamic model at pressures p≲ 2bar . As all models are in line with the ideal gas law, we hypothesize the presence of real gas effects in the measured spectra.

  20. Determination of surface normal temperature gradients using thermographic phosphors and filtered Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Brübach, J.; Zetterberg, J.; Omrane, A.; Li, Z. S.; Aldén, M.; Dreizler, A.

    2006-09-01

    Wall temperature as well as the temperature distribution within or close-by the boundary layer of an electrically heated axisymmetric jet impinging on a flat plate were monitored to deduce wall-normal temperature gradients. The radial surface temperature profile of the plate was determined by coating it with thermographic phosphors (TPs), materials whose phosphorescence decay time is dependent on their temperature. The TP was excited electronically by a frequency-tripled Nd:YAG laser (355 nm) and the temporal decay of the phosphorescence intensity was measured zero-dimensionally by a photomultiplier tube. In this case the 659-nm emission line of Mg3F2GeO4:Mn was monitored. The non-intrusive measurement of gas temperatures near the surface was performed two-dimensionally by filtered Rayleigh scattering (FRS). A tunable frequency-tripled single-longitudinal-mode alexandrite laser beam at 254 nm was formed into a light sheet pointing parallel to the surface. The scattered light was imaged through a very narrow linewidth atomic mercury filter onto an intensified charged coupled device (ICCD). The elastic stray light from surfaces was strongly suppressed, whereas Doppler-broadened light was detected. Thermographic phosphors proved to be reliable for the measurement of surface temperatures. Dependent on the specific experimental conditions, problems appeared with signals interfering with the FRS radiation close-by the surface. Results and challenges of this approach are discussed.

  1. Absolute Rayleigh scattering cross sections of gases and freons of stratospheric interest in the visible and ultraviolet regions

    NASA Technical Reports Server (NTRS)

    SHARDANAND; Rao, A. D. P.

    1977-01-01

    The laboratory measurements of absolute Rayleigh scattering cross sections as a function wavelength are reported for gas molecules He, Ne, Ar, N2, H2, O2, CO2, CH4 and for vapors of most commonly used freons CCl2F2, CBrF3, CF4, and CHClf2. These cross sections are determined from the measurements of photon scattering at an angle of 54 deg 44 min which yield the absolute values independent of the value of normal depolarization ratios. The present results show that in the spectral range 6943-3638A deg, the values of the Rayleigh scattering cross section can be extrapolated from one wavelength to the other using 1/lambda (4) law without knowing the values of the polarizabilities. However, such an extrapolation can not be done in the region of shorter wavelengths.

  2. Multiple-Rayleigh-scatterer-induced mode splitting in a high-Q whispering-gallery-mode microresonator

    SciTech Connect

    Yi Xu; Xiao Yunfeng; Liu Yongchun; Li Beibei; Chen Youling; Li Yan; Gong Qihuang

    2011-02-15

    We theoretically investigate the mode-splitting phenomenon in a high-Q whispering-gallery-mode (WGM) microresonator coupled to multiple subwavelength Rayleigh scatterers. It is shown that the phase factors of the WGMs play the central role in such a system. Unlike the single-scatterer case, these phase factors in a multiscatterer system significantly influence both the modal coupling strength and the scattering-induced loss of a pair of counterpropagating WGMs. We scrutinize the condition for observing the splitting of transmission spectra. The mechanism can be used for highly sensitive biosensing, and the size of nanoparticles that can be detected is extended down to tens of nanometers.

  3. Molecular Rayleigh Scattering Diagnostic for Measurement of High Frequency Temperature Fluctuations

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.

    2005-01-01

    A novel technique for measurement of high frequency temperature fluctuations in unseeded gas flows using molecular Rayleigh scattering is investigated. The spectrum of laser light scattered from molecules in a gas flow is resolved using a Fabry-Perot interferometer. The width of the spectral peak is broadened by thermal motion of the molecules and hence is related to gas temperature. The interference fringe pattern containing spectral information is divided into four concentric regions using a series of mirrors angled with respect to one another. Light from each of these regions is directed towards photomultiplier tubes and sampled at 10 kHz using photon counting electronics. Monitoring the relative change in intensity within each region allows measurement of gas temperature. Independently monitoring the total scattered intensity provides a measure of gas density. This technique also has the potential to simultaneously measure a single component of flow velocity by monitoring the spectral peak location. Measurements of gas temperature and density are demonstrated using a low speed heated air jet surrounded by an unheated air co-flow. Mean values of temperature and density are shown for radial scans across the jet flow at a fixed axial distance from the jet exit plane. Power spectra of temperature and density fluctuations at several locations in the jet are also shown. The instantaneous measurements have fairly high uncertainty; however, long data records provide highly accurate statistically quantities, which include power spectra. Mean temperatures are compared with thermocouple measurements as well as the temperatures derived from independent density measurements. The accuracy for mean temperature measurements was +/- 7 K.

  4. Comparison of Coincident Rayleigh-Scatter and Sodium Resonance Lidar Temperature Measurements from the Mesosphere-Lower-Thermosphere Region

    NASA Astrophysics Data System (ADS)

    Sox, L.; Wickwar, V. B.; Yuan, T.; Criddle, N.

    2015-12-01

    There are relatively few instruments that have the capabilities to make near continuous measurements of the mesosphere-lower-thermosphere (MLT) region. Rayleigh scatter and resonance lidars, particularly sodium resonance lidar, have been the two dominant ground-based techniques for acquiring mesosphere and MLT vertical temperature profiles, respectively, for more than two decades. With these measurements, the dynamics (gravity waves, tides) and long-term temperature trends (upper atmosphere cooling) of the MLT region can be studied. The Utah State University (USU; 41.7º N, 111.8º W) campus hosts a unique upper atmospheric observatory which houses both a high-power, large-aperture Rayleigh lidar and a sodium resonance Doppler lidar. For the first time, we will present coordinated, night-time averaged temperatures, overlapping in observational range (80-110 km), from the two lidars. This overlap has been achieved through the relocation of the sodium lidar from Colorado State University to USU's campus and through upgrades to the existing USU Rayleigh lidar which elevated its observational range from 45-90 km to 70-115 km. The comparison of the two sets of temperature measurements is important because the two lidar techniques derive temperature profiles using different scattering processes and analysis methods. Furthermore, previous climatological comparisons, between Rayleigh and sodium lidar, [Argall and Sica, 2007] have suggested that significant temperature differences can occur. This comparison aims to explore possible temperature effects from the differences in the two measurement techniques.

  5. Coupling of a single diamond nanocrystal to a whispering-gallery microcavity: Photon transport benefitting from Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Liu, Yong-Chun; Xiao, Yun-Feng; Li, Bei-Bei; Jiang, Xue-Feng; Li, Yan; Gong, Qihuang

    2011-07-01

    We study the Rayleigh scattering induced by a diamond nanocrystal in a whispering-gallery-microcavity-waveguide coupling system and find that it plays a significant role in the photon transportation. On the one hand, this study provides insight into future solid-state cavity quantum electrodynamics aimed at understanding strong-coupling physics. On the other hand, benefitting from this Rayleigh scattering, effects such as dipole-induced transparency and strong photon antibunching can occur simultaneously. As a potential application, this system can function as a high-efficiency photon turnstile. In contrast to B. Dayan [ScienceSCIEAS0036-807510.1126/science.1152261 319, 1062 (2008)], the photon turnstiles proposed here are almost immune to the nanocrystal’s azimuthal position.

  6. Coupling of a single diamond nanocrystal to a whispering-gallery microcavity: Photon transport benefitting from Rayleigh scattering

    SciTech Connect

    Liu Yongchun; Xiao Yunfeng; Li Beibei; Jiang Xuefeng; Li Yan; Gong Qihuang

    2011-07-15

    We study the Rayleigh scattering induced by a diamond nanocrystal in a whispering-gallery-microcavity-waveguide coupling system and find that it plays a significant role in the photon transportation. On the one hand, this study provides insight into future solid-state cavity quantum electrodynamics aimed at understanding strong-coupling physics. On the other hand, benefitting from this Rayleigh scattering, effects such as dipole-induced transparency and strong photon antibunching can occur simultaneously. As a potential application, this system can function as a high-efficiency photon turnstile. In contrast to B. Dayan et al. [Science 319, 1062 (2008)], the photon turnstiles proposed here are almost immune to the nanocrystal's azimuthal position.

  7. Measurement of the thermal diffusivity of liquids by the forced Rayleigh scattering method: Theory and experiment

    NASA Astrophysics Data System (ADS)

    Nagasaka, Y.; Hatakeyama, T.; Okuda, M.; Nagashima, A.

    1988-07-01

    This article is devoted to the theory and experiment of the forced Rayleigh scattering method for measurement of thermal diffusivity of liquids which can be employed in the form of an instrument operated optically in a contact-free manner. The theoretical considerations included are: (1) effect of cell wall, (2) effect of dye, (3) effect of Gaussian beam intensity distribution, (4) effect of heating duration time, and (5) effect of coupled dye and wall for a heavily absorbing sample. The errors caused by inadequate setting of optical conditions are also analyzed: (1) effects of grating thickness and (2) effects of initial temperature amplitude. Experimental verifications of the theory have been carried out through the measurements on toluene and water as standard reference substances. As a result of these experiments and theory, the criteria for optimum measuring conditions became available. To demonstrate the applicability of the present theory and the apparatus, the thermal diffusivities of toluene and methanol have been measured near room temperature under atmospheric pressure. The accuracy of the present measurement is estimated to be ±3%.

  8. Highly sensitive ratiometric quantification of cyanide in water with gold nanoparticles via Resonance Rayleigh Scattering.

    PubMed

    Hernández, Yulán; Coello, Yves; Fratila, Raluca M; de la Fuente, Jesús M; Lionberger, Troy A

    2017-05-15

    A highly sensitive and selective ratiometric sensor for the quantification of cyanide (CN(-)) in aqueous samples has been developed using spherical gold nanoparticles (AuNPs) stabilized by polysorbate 40 (PS-40). Three different AuNP sizes (14, 40 and 80nm mean diameters) were used to evaluate the response of the sensor using both colorimetric and Resonance Rayleigh Scattering (RRS) detection schemes. The best results were obtained for the sensor using 40nm AuNPs, for which the limits of detection (LODs) were found to be 100nmolL(-1) in a benchtop instrument and 500nmolL(-1) by the naked eye, values well below the maximum acceptable level for drinking water (1.9µmolL(-1)) set by the World Health Organization (WHO). The practical use of the 40nm-AuNPs RRS sensor was demonstrated with the determination of CN(-) in drinking and fresh waters. Finally, the sensor was successfully implemented in a compact portable device consisting of two light-emitting diodes (LEDs) and a miniature spectrometer, turning this sensor into a very potent tool for its application as a quick routine field-deployable analytical method.

  9. Rayleigh Scattering Density Measurements, Cluster Theory, and Nucleation Calculations at Mach 10

    NASA Technical Reports Server (NTRS)

    Balla, R. Jeffrey; Everhart, Joel L.

    2012-01-01

    In an exploratory investigation, quantitative unclustered laser Rayleigh scattering measurements of density were performed in the air in the NASA Langley Research Center's 31 in. Mach 10 wind tunnel. A review of 20 previous years of data in supersonic and Mach 6 hypersonic flows is presented where clustered signals typically overwhelmed molecular signals. A review of nucleation theory and accompanying nucleation calculations are also provided to interpret the current observed lack of clustering. Data were acquired at a fixed stagnation temperature near 990Kat five stagnation pressures spanning 2.41 to 10.0 MPa (350 to 1454 psi) using a pulsed argon fluoride excimer laser and double-intensified charge-coupled device camera. Data averaged over 371 images and 210 pixels along a 36.7mmline measured freestream densities that agree with computed isentropic-expansion densities to less than 2% and less than 6% at the highest and lowest densities, respectively. Cluster-free Mach 10 results are compared with previous clustered Mach 6 and condensation-free Mach 14 results. Evidence is presented indicating vibrationally excited oxygen and nitrogen molecules are absorbed as the clusters form, release their excess energy, and inhibit or possibly reverse the clustering process. Implications for delaying clustering and condensation onset in hypersonic and hypervelocity facilities are discussed.

  10. Hydride generation-resonance Rayleigh scattering and SERS spectral determination of trace Bi.

    PubMed

    Liang, Xiaojing; Wen, Guiqing; Liu, Qingye; Liang, Aihui; Jiang, Zhiliang

    2016-09-05

    In acidic solutions, Bi(III) was reduced by NaBH4 to form BiH3 gas. Using I3(-)graphene oxide (GO) as absorption solution, the BiH3 gas reacted with I3(-) to form I(-) that resulted in the I3(-) concentration decreasing. In the absence of BiH3, the I3(-) concentration was high, and as receptors it was closed to the surfaces of GO which was as donors. Then the surface plasmon resonance Rayleigh scattering (RRS) energy of GO transfers to I3(-) heavily, and results in the RRS quenching severely. With the increase of the Bi(III) concentration, the receptors and the RRS energy transfer (RRS-ET) decreased, so the RRS intensity enhanced linearly at 370nm. The RRS intensity was linear to the Bi(III) concentration in 0.05-5.5μmol/L, with a detection limit of 4ng/mL Bi. A new RRS-ET spectral method was developed for the determination of trace Bi(III). Using I3(-) as the absorption solution, silver nanorod (AgNR) as sol substrate and Vitoria blue B (VBB) as molecular probe, a SERS method was developed for detection of Bi.

  11. Gold Nanorod Based Selective Identification of Escherichia coli Bacteria Using Two-Photon Rayleigh Scattering Spectroscopy.

    PubMed

    Singh, Anant K; Senapati, Dulal; Wang, Shuguang; Griffin, Jelani; Neely, Adria; Candice, Perry; Naylor, Khaleah M; Varisli, Birsen; Kalluri, Jhansi Rani; Ray, Paresh Chandra

    2009-07-28

    The presence of E. coli in foodstuffs and drinking water is a chronic worldwide problem. The worldwide food production industry is worth about U.S. $578 billion, and the demand for biosensors to detect pathogens and pollutants in foodstuffs is growing day by day. Driven by the need, we report for the first time that two-photon Rayleigh scattering (TPRS) properties of gold nanorods can be used for rapid, highly sensitive and selective detection of Escherichia coli bacteria from aqueous solution, without any amplification or enrichment in 50 colony forming units (cfu)/mL level with excellent discrimination against any other bacteria. TPRS intensity increases 40 times when anti- E. coli antibody-conjugated nanorods were mixed with various concentrations of Escherichia coli O157:H7 bacterium. The mechanism of TPRS intensity change has been discussed. This bionanotechnology assay could be adapted in studies using antibodies specific for various bacterial pathogens for the detection of a wide variety of bacterial pathogens used as bioterrorism agents in food, clinical samples, and environmental samples.

  12. Resonance Rayleigh scattering method for highly sensitive detection of chitosan using aniline blue as probe

    NASA Astrophysics Data System (ADS)

    Zhang, Weiai; Ma, Caijuan; Su, Zhengquan; Bai, Yan

    2016-11-01

    This paper describes a highly sensitive and accurate approach using aniline blue (AB) (water soluble) as a probe to determine chitosan (CTS) through Resonance Rayleigh scattering (RRS). Under optimum experimental conditions, the intensities of RRS were linearly proportional to the concentration of CTS in the range from 0.01 to 3.5 μg/mL, and the limit of detection (LOD) was 6.94 ng/mL. Therefore, a new and highly sensitive method based on RRS for the determination of CTS has been developed. Furthermore, the effect of molecular weight of CTS and the effect of the degree of deacetylation of CTS on the accurate quantification of CTS was studied. The experimental data was analyzed by linear regression analysis, which indicated that the molecular weight and the degree of deacetylation of CTS had no statistical significance and this method could be used to determine CTS accurately. Meanwhile, this assay was applied for CTS determination in health products with satisfactory results.

  13. Resonance Rayleigh scattering method for the determination of cationic surfactants with chromium(VI)-iodide system.

    PubMed

    Liu, Shaopu; Shi, Yan; Liu, Zhongfang; Luo, Hongqun; Kong, Ling

    2006-05-01

    A method for detecting and identifying cationic surfactant in some chemical samples for daily use that include Head & Shoulder Ampoule and Slek Shower Lotion has been developed. In an acid medium, chromium(VI) oxidizes I(-) to produce I(2), I(2) binds excess of I(-) to form I(3)(-), and I(3)(-) can further react with a cationic surfactant (CS) (such as cetyldimethyl benzylammonium chloride (CDBAC), Zephiramine (Zeph), cetylpyridinium bromide (CPB), tetradecyl pyridinium bromide (TPB) and cetyltrimethylammonium bromide (CTAB)) to form ion-association complexes [CS][I(3)]. This results in a significant enhancement of resonance Rayleigh scattering (RRS) and appearance of new RRS spectra. The RRS spectral characteristics of the ion-association complexes, the influencing factors and the optimum conditions of the reactions have been investigated. The intensities of RRS are directly proportional to the concentration of CS. CS in samples are collected using a treated anion exchange column and subsequently complexed by I(3)(-); then the RRS intensities of CS complex are determined at 495 nm. The reactions have high sensitivities, and their detection limits are 7.05 - 9.62 ng/mL for different CS. The effects of foreign substances are investigated and the results show that the method has good selectivity.

  14. Spectrally- and polarization-resolved hyper-Rayleigh scattering measurements with polarization-insensitive detection

    NASA Astrophysics Data System (ADS)

    Němec, P.; Pásztor, F.; Brajer, M.; Němec, I.

    2017-04-01

    Determination of the molecular first hyperpolarizability by hyper-Rayleigh scattering (HRS) is usually significantly complicated by a presence of the multiphoton excited fluorescence which has to be separated from HRS to obtain a meaningful values of the hyperpolarizability. We show, by performing a spectrally-resolved measurement, that the intensity and spectral shape of the fluorescence can depend strongly on the fundamental laser wavelength. Consequently, a properly selected excitation wavelength can significantly simplify the process of separation of HRS from the detected signal. We tested the developed experimental setup with a polarization-insensitive detection by measuring HRS generated in water and in aqueous solutions of 2-aminopyrimidine (AMP) and its monocation (HAMP). The effective hyperpolarizability of AMP and HAMP was measured experimentally and compared with that obtained by quantum chemical calculations. The polarization-resolved HRS measurement was performed for AMP and the experimentally obtained depolarization ratio agrees well with that predicted theoretically, which confirms that routine density functional theory computations of static hyperpolarizability tensor components can be considered as a sufficient approach suitable for non-interacting molecules dissolved in water.

  15. Rayleigh light scattering detection of three α1-adrenoceptor antagonists coupled with high performance liquid chromatograph

    NASA Astrophysics Data System (ADS)

    Li, Ai Ping; Peng, Huanjun; Peng, Jing Dong; Zhou, Ming Qiong; Zhang, Jing

    2015-08-01

    Herein, a Rayleigh light-scattering (RLS) detection method combined with high performance liquid chromatograph (HPLC) without any post-column probe was developed for the separation and determination of three α1-adrenoceptor antagonists. The quantitative analysis is benefiting from RLS signal enhancement upon addition of methanol which induced molecular aggregation to form an hydrophobic interface between aggregates and water that produce a sort of superficial enhanced scattering effect. A good chromatographic separation among the compounds was achieved using a Gemini 5u C18 reversed phase column (250 mm × 4.6 mm; 4 μm) with a mobile phase consisting of methanol and ammonium acetate-formic acid buffer solution (25 mM; pH = 3.0) at the flow rate of 0.7 mL min-1. The RLS signal was monitored at λex = λem = 354 nm. A limit of detection (LOD) of 0.065-0.70 μg L-1 was reached and a linear range was found between peak height and concentration in the range of 0.75-15 μg L-1 for doxazosin mesylate (DOX), 0.075-3.0 μg L-1 for prazosin hydrochloride (PRH), and 0.25-5 μg L-1 for terazosin hydrochloride (TEH), with linear regression coefficients all above 0.999. Recoveries from spiked urine samples were 88.4-99.0% which is within acceptable limits. The proposed method is convenient, reliable and sensitive which has been used successfully in human urine samples.

  16. Rayleigh Scattering Diagnostic Used to Measure Velocity and Density Fluctuation Spectra

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Panda, Jayanta; Elam, Kristie A.

    2003-01-01

    A new, molecular Rayleigh-scattering-based flow diagnostic developed at the NASA Glenn Research Center has been used for the first time to measure the power spectrum of both gas density and radial velocity components in the plumes of high-speed jets. The objective of the work is to develop an unseeded, nonintrusive dynamic measurement technique for studying turbulent flows in NASA test facilities. This technique provides aerothermodynamic data not previously obtainable. It is particularly important for supersonic flows, where hot wire and pitot probes are difficult to use and disturb the flow under study. The effort is part of the nonintrusive instrumentation development program supporting propulsion research at the NASA Glenn Research Center. In particular, this work is measuring fluctuations in flow velocity, density, and temperature for jet noise studies. These data are valuable to researchers studying the correlation of flow fluctuations with far-field noise. One of the main objectives in jet noise research is to identify noise sources in the jet and to determine their contribution to noise generation. The technique is based on analyzing light scattered from molecules within the jet using a Fabry-Perot interferometer operating in a static imaging mode. The PC-based data acquisition system can simultaneously sample velocity and density data at rates to about 100 kHz and can handle up to 10 million data records. We used this system to interrogate three different jet nozzle designs in a Glenn free-jet facility. Each nozzle had a 25.4-mm exit diameter. One was convergent, used for subsonic flow measurements and to produce a screeching underexpanded jet with a fully expanded Mach number of 1.42. The other nozzles (Mach 1.4 and 1.8) were convergent-divergent types. The radial component of velocity and gas density were simultaneously measured in this work.

  17. High performance liquid chromatography coupled with resonance Rayleigh scattering for the detection of three fluoroquinolones and mechanism study

    NASA Astrophysics Data System (ADS)

    Zhou, Mingqiong; Peng, Jingdong; He, Rongxing; He, Yuting; Zhang, Jing; Li, Aiping

    2015-02-01

    A reliable and versatile high performance liquid chromatography coupled with resonance Rayleigh scattering method was established for the determination of three fluoroquinolones, including levofloxacin, norfloxacin and enrofloxacin in water sample and human urine sample. In pH 4.4-4.6 Britton-Robinson buffer medium, the fluoroquinolones separated by high performance liquid chromatography could react with erythrosine to form 1:1 ion-association complexes, which could make contributions to the great enhancement of RRS. The resonance Rayleigh scattering signal was recorded at λex = λem = 330 nm. The resonance Rayleigh scattering spectral characteristics of the drugs and the experimental conditions such as pH, detection wavelength, erythrosine concentration, flow rate, the length of reaction tube were studied. Quantum chemistry calculation, Fourier transform infrared spectroscopy and absorption spectroscopy were used to discuss the reaction mechanism. The recoveries of samples added standard ranged from 97.53% to 102.00%, and the relative standard deviation was below 4.64%. The limit of detection (S/N = 3) of 0.05-0.12 μg mL-1 was reached, and the linear regression coefficients were all above 0.999. The proposed method was proved as a simple, low cost and high sensitivity method.

  18. High performance liquid chromatography coupled with resonance Rayleigh scattering for the detection of three fluoroquinolones and mechanism study.

    PubMed

    Zhou, Mingqiong; Peng, Jingdong; He, Rongxing; He, Yuting; Zhang, Jing; Li, Aiping

    2015-02-05

    A reliable and versatile high performance liquid chromatography coupled with resonance Rayleigh scattering method was established for the determination of three fluoroquinolones, including levofloxacin, norfloxacin and enrofloxacin in water sample and human urine sample. In pH 4.4-4.6 Britton-Robinson buffer medium, the fluoroquinolones separated by high performance liquid chromatography could react with erythrosine to form 1:1 ion-association complexes, which could make contributions to the great enhancement of RRS. The resonance Rayleigh scattering signal was recorded at λex=λem=330 nm. The resonance Rayleigh scattering spectral characteristics of the drugs and the experimental conditions such as pH, detection wavelength, erythrosine concentration, flow rate, the length of reaction tube were studied. Quantum chemistry calculation, Fourier transform infrared spectroscopy and absorption spectroscopy were used to discuss the reaction mechanism. The recoveries of samples added standard ranged from 97.53% to 102.00%, and the relative standard deviation was below 4.64%. The limit of detection (S/N=3) of 0.05-0.12 μg mL(-1) was reached, and the linear regression coefficients were all above 0.999. The proposed method was proved as a simple, low cost and high sensitivity method.

  19. A novel method for the determination of fast green in grape wine based on resonance Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    Li, Qin; Tan, Xuanping; Zheng, Xiaobo; Tang, Weiwei; Yang, Jidong

    2015-11-01

    A novel resonance Rayleigh scattering method was developed for the determination of fast green (FCF) in grape wine. In pH 2.5 Britton Robinson (BR) buffer solution, the scattering signal of acridine orange (AO) was remarkably enhanced after adding trace amount of FCF and forming an ion-association complex, which not only resulted in the change of absorption spectrum, fluorescence spectra, but also led to a significant enhancement of resonance Rayleigh scattering (RRS), frequency doubling scattering (FDS), and second order scattering (SOS). The linear ranges and detection limits for RRS, SOS and FDS were 2-45 × 10-6 mol L-1, 2-24 × 10-6 mol L-1, 2-20 × 10-6 mol L-1, and 8.0 × 10-8 mol L-1, 4.7 × 10-7 mol L-3, 1.0 × 10-7 mol L-3, respectively. In this work, the optimum conditions, the influencing factors and the effects of coexisting substances on the reaction were investigated. The method can be applied to the determination of FCF in grape wine and the results were satisfactory.

  20. Accuracy of RGD approximation for computing light scattering properties of diffusing and motile bacteria. [Rayleigh-Gans-Debye

    NASA Technical Reports Server (NTRS)

    Kottarchyk, M.; Chen, S.-H.; Asano, S.

    1979-01-01

    The study tests the accuracy of the Rayleigh-Gans-Debye (RGD) approximation against a rigorous scattering theory calculation for a simplified model of E. coli (about 1 micron in size) - a solid spheroid. A general procedure is formulated whereby the scattered field amplitude correlation function, for both polarized and depolarized contributions, can be computed for a collection of particles. An explicit formula is presented for the scattered intensity, both polarized and depolarized, for a collection of randomly diffusing or moving particles. Two specific cases for the intermediate scattering functions are considered: diffusing particles and freely moving particles with a Maxwellian speed distribution. The formalism is applied to microorganisms suspended in a liquid medium. Sensitivity studies revealed that for values of the relative index of refraction greater than 1.03, RGD could be in serious error in computing the intensity as well as correlation functions.

  1. Comparison of Gas Displacement based on Thermometry in the Pulse Tube with Rayleigh Scattering

    NASA Astrophysics Data System (ADS)

    Hagiwara, Yasumasa; Nara, Kenichi; Ito, Seitoku; Saito, Takamoto

    A pulse tube refrigerator has high reliability because of its simple structure. Recently the level of development activity of the pulse tube refrigerator has increased, but the quantitative understanding of the refrigeration mechanism has not fully been obtained. Therefore various explanations were proposed. The concept of virtual gas piston in particular helps us to understand the function of a phase shifter such as a buffer tank and an orifice because the virtual gas piston corresponds to a piston of a Stirling refrigerator. However it is difficult to directly measure the averaged gas displacement which corresponds to the virtual gas piston because uniform gas flow such as a gas piston does not always exist. For example, there are a jet flow from orifice and circulated flows in a pulse tube, which are predicted theoretically. In spite of these phenomena, the averaged gas displacement is very important in practical use because it can simply predict the performance from the displacement. In this report, we calculate the averaged gas displacement and mass flow through an orifice. The mass flow is calculated from the pressure change in a buffer tank. The averaged gas displacement is calculated from temperature profiles in the pulse tube and the mass flow. It is necessary to measure temperature in the pulse tube as widely as possible in order to calculate the averaged gas displacement. We apply a method using the Rayleigh Scattering the thermometry in the pulse tube. With this method, it is possible to perform 2-dimensional measurement without disturbing the gas flow. By this method, the averaged gas displacements and the temperature profiles of basic and orifice types of refrigeration were compared.

  2. SEARCH FOR RAYLEIGH SCATTERING IN THE ATMOSPHERE OF GJ1214b

    SciTech Connect

    De Mooij, E. J. W.; Jayawardhana, R.; Brogi, M.; Snellen, I. A. G.; Hoekstra, H.; Otten, G. P. P. L.; Bekkers, D. H.; Haffert, S. Y.; Van Houdt, J. J.; De Kok, R. J.; Croll, B.

    2013-07-10

    We investigate the atmosphere of GJ1214b, a transiting super-Earth planet with a low mean density, by measuring its transit depth as a function of wavelength in the blue optical portion of the spectrum. It is thought that this planet is either a mini-Neptune, consisting of a rocky core with a thick, hydrogen-rich atmosphere, or a planet with a composition dominated by water. Most observations favor a water-dominated atmosphere with a small scale-height, however, some observations indicate that GJ1214b could have an extended atmosphere with a cloud layer muting the molecular features. In an atmosphere with a large scale-height, Rayleigh scattering at blue wavelengths is likely to cause a measurable increase in the apparent size of the planet toward the blue. We observed the transit of GJ1214b in the B band with the FOcal Reducing Spectrograph at the Very Large Telescope and in the g band with both ACAM on the William Herschel Telescope (WHT) and the Wide Field Camera at the Isaac Newton Telescope (INT). We find a planet-to-star radius ratio in the B band of 0.1162 {+-} 0.0017, and in the g band 0.1180 {+-} 0.0009 and 0.1174 {+-} 0.0017 for the WHT and INT observations, respectively. These optical data do not show significant deviations from previous measurements at longer wavelengths. In fact, a flat transmission spectrum across all wavelengths best describes the combined observations. When atmospheric models are considered, a small scale-height water-dominated model fits the data best.

  3. Coherent Rayleigh-Brillouin scattering for in situ detection of nanoparticles and large molecules in gas and plasma

    NASA Astrophysics Data System (ADS)

    Gerakis, A.; Shneider, M. N.; Stratton, B. C.; Santra, B.; Car, R.; Raitses, Y.

    2016-09-01

    Laser-based diagnostics methods, such as Spontaneous and Coherent Rayleigh and Rayleigh-Brillouin scattering (SRBS and CRBS), can be used for in-situ detection and characterization of nanoparticle shape and size as well as their concentration in an inert gas atmosphere. We recently developed and tested this advanced diagnostic at PPPL. It was shown that the signal intensity of the CRBS signal depends on the gas-nanoparticle mixture composition, density and the polarizabilities of the mixture components. The measured results agree well with theoretical predictions of Refs. In this work, we report the application of this diagnostic to monitor nucleation and growth of nanoparticles in a carbon arc discharge. In support of these measurements, A time-dependent density functional theory was used to compute the frequency-dependent polarizabilities of various nanostructures in order to predict the corresponding Rayleigh scattering intensities as well as light depolarization. Preliminary results of measurements demonstrate that CRBS is capable to detect nanoparticles in volume. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division.

  4. Pushing the upper limit of Rayleigh-scatter Temperatures Retrievals into the Lower Thermosphere Using an Inversion Approach

    NASA Astrophysics Data System (ADS)

    Bandoro, J.; Sica, R. J.; Argall, S.

    2012-12-01

    An important aspect of solar terrestrial relations is the coupling between the lower and upper atmosphere-ionosphere system. The coupling is evident in the general circulation of the atmosphere, where waves generate in the lower atmosphere play an important role in the dynamics of the upper atmosphere, which feeds back on the lower atmosphere's circulation. To address coupling problems requires measurements over the broadest range of heights possible. A recently developed retrieval method for temperature profiles from Rayleigh-scatter lidar measurements using an inversion approach allows the upward extension of the altitude range of temperature by 10 to 15 km over the conventional method, thus producing the equivalent of increasing the systems power-aperture product by 4 times [1]. The method requires no changes to the lidar's hardware and thus, can be applied to the body of existing measurements. In addition, since the uncertainties of the retrieved temperature profile are found by a Monte Carlo error analysis, it is possible to isolate systematic and random uncertainties to model the effect of each one on the final uncertainty product for the temperature profile. This unambiguous separation of uncertainties was not previously possible as only the propagation of the statistical uncertainties are typically reported. For the Purple Crow Lidar, corrections for saturation (e.g. non-linearity) in the photocount returns, ozone extinction and background removal all contribute to the overall systematic uncertainty. Results of individually varying each systematic correction and the effect on the final temperature uncertainty through Monte Carlo realizations are presented to determine the importance for each one. For example, it was found that treatment of the background correction as a systematic versus statistical uncertainty gave results in agreement with each other. This new method is then applied to measurements obtained by the Purple Crow lidar' Rayleigh-scatter

  5. Improvement in Suppression of Pulsed Nd:YAG Laser Light With Iodine Absorption Cells for Filtered Rayleigh Scattering Measurements

    NASA Technical Reports Server (NTRS)

    Seasholtz, Richard G.; Buggele, Alvin E

    1997-01-01

    Filtered Rayleigh scattering using iodine absorption cells is an effective technique for obtaining density, temperature, and velocity measurements in high speed confined flows. By tuning a single frequency laser to a strong iodine absorption line, stray scattered laser light can be greatly suppressed. For example, the minimum transmission predicted by an iodine absorption model calculation is less than 10(exp -5) at the 18788.44/cm line using a 200 mm absorption cell containing iodine vapor at 0.46 T. Measurements obtained by other researches using a CW Nd:YAG laser agree with the model calculations. However, measurements made by us and by others using Q-switched, injection-seeded, frequency doubled Nd:YAG lasers only show minimum transmission of about 3 x 10(exp -3). This greatly reduces the applicability of the filtered Rayleigh scattering technique using these lasers in experiments having large amounts of stray scattered laser light. The purposes of the present study are to characterize the spectrum of the excess light transmitted by the iodine cell and to make changes to the laser to reduce the transmitted laser light. Transmission data as a function of laser frequency for the iodine absorption line at 18788.44/cm are presented. A planar mirror Fabry-Perot interferometer was used to characterize the frequency spectrum of the light passed through the cell. Measurements taken with the laser tuned to the center of the iodine absorption line show the light transmitted through the iodine cell to have a component with a bandwidth of about 40 GHz. This is probably caused by other modes in the laser that exist in spite of the single frequency injection beam. A second broadband component was also observed, possibly caused by the laser flash lamps or by fluorescence. An intracavity etalon was installed in the laser oscillator cavity to suppress the 40 GHz component. Measurements taken with the etalon tuned to the injection frequency showed a reduction in the transmitted

  6. Blue Skies through a Blue Sky: an attempt to detect Rayleigh scattering in an exoplanet atmosphere from a ground-based telescope

    NASA Astrophysics Data System (ADS)

    Luchsinger, Kristen; Redfield, Seth; Cauley, Paul W.; Barman, Travis S.; Jensen, Adam G.

    2017-01-01

    When studying planetary atmospheres, scattering signatures, such as Rayleigh scattering, can often be the most easily characterized signal. This is especially true in terrestrial atmospheres, where Rayleigh scattering is the dominant spectral feature in optical wavelengths. These scattering signatures, unlike molecular or atomic line absorption, are broad and continuous, and are char- acterized by a single slope. Rayleigh scattering provides an imporant glimpse into the atmospheric composition of an exoplanet's atmosphere, and a Rayleigh scattering detection on a smaller, ground-based telescope can be a useful method to identify interesting science targets for larger, space-based telescopes.We will present observations of three exoplanets using the HYDRA multi- object spectrometer on the WIYN telescope at Kitt Peak National Observatory. We obtained two transits each for WASP 12b and GJ 3470b, and one transit for HD 189733b, for a range of wavelengths between 4500 Å and 9201 Å. A successful Rayleigh scattering detection in the atmospheres of these planets using this in- strument would represent a step forward in our current detection capabilities and open up the study of planetary atmospheres to smaller, ground-based telescopes.Data presented herein were obtained at the WIYN Observatory from telescope time allocated to NN-EXPLORE through the scientific partnership of the National Aeronautics and Space Administration, the National Science Foundation, and the National Optical Astronomy Observatory. This work was supported by a NASA WIYN PI Data Award, administered by the NASA Exoplanet Science Institute.

  7. [Determination of Trace Boron Based on Gold Nanorod Plasmonic Resonance Rayleigh Scattering Energy Transfer to the Coordinate].

    PubMed

    Ye, Ling-ling; Li, Ting-sheng; Luo, Yang-he; Wen, Gui-qing; Liang, Ai-hui; Jiang, Zhi-liang

    2015-05-01

    B is a necessary trace element for human and animals, but the excess intake of B caused poison. Thus, it is very important to determination of B in foods and water. The target of this study is development of a new, sensitive and selective resonance Rayleigh scattering energy transfer (RRS-ET) for the determination of B. The combination of energy transfer with resonance Rayleigh scattering (RRS) has developed a new technology called RRS-ET, which can realize selective and sensitive detection of boric acid. The gold nanorods in diameter of 12 nm and length of 37 nm were prepared by the seed growth procedure. In pH 5. 6 NH4 Ac-HAc buffer solution and in the presence of azomethine-H (AMH), the gold nanorod particles exhibited a strong resonance Rayleigh scattering (RRS) peak at 404 nm. In the presence of boric acid, it reacts with AMH to form AMH-boric acid (AMH-B) complexes. When the complexe as a receptor close to the gold nanorod as a donor, the resonance Rayleigh scattering energy transfer (RRS-ET) take placed that resulted in the Rayleigh scattering signal quenching. With the increase of the concentration of boric acid, the formed complexes increased, the scattering light energy of gold nanorod transfer to the complexes increased, resulting in the Rayleigh scattering intensity linearly reduced at 404 nrn. The decreased RRS intensity responds linearly to the concentration of boron over 10~750 ng . mL-1 B, with a regress equation of ΔI404 nm =3. 53c+24 and a detection of 5 ng mL-1 B. The influence of coexistence substances on the RRS-ET determination of 2. 3 X 10(-7) mol . L-1 B was considered in details. Results showed that this new RRS-ET method is of high selectivity, that is, 4 X 10(-4) mol . L-1 Mn2+, Cd2+, Zn2+, Bi+, Na+, Al3+, glucose, Hg2+, IO3-, F-, SO(2-)3, SiO3-, NO3-, CIO4-, H2O2, mannitol, glycerol, and ethylene glycol, 4X 10(-5) mol . L-1 L-tyrosine, and 2 X 10(-4) mol . L-1 L-glutamic acid do not interfere with the determination. Based on this, a new

  8. Study on the interaction between fluoroquinolones and erythrosine by absorption, fluorescence and resonance Rayleigh scattering spectra and their application

    NASA Astrophysics Data System (ADS)

    Wang, Jian; Liu, Zhongfang; Liu, Jiangtao; Liu, Shaopu; Shen, Wei

    2008-03-01

    In pH 4.4-4.5 Britton-Robinson (BR) buffer solution, fluoroquinolone antibiotics (FLQs) including ciprofloxacin (CIP), norfloxacin (NOR), levofloxacin (LEV) and lomefloxacin (LOM) could react with erythrosine (Ery) to form 1:1 ion-association complexes, which not only resulted in the changes of the absorption spectra and the quenching of fluorescence, but also resulted in the great enhancement of resonance Rayleigh scattering (RRS). These offered some indications of the determination of fluoroquinolone antibiotics by spectrophotometric, fluorescence and resonance Rayleigh scattering methods. The detection limits for fluoroquinolone antibiotics were in the range of 0.097-0.265 μg/mL for absorption methods, 0.022-0.100 μg/mL for fluorophotometry and 0.014-0.027 μg/mL for RRS method, respectively. Among them, the RRS method had the highest sensitivity. In this work, the spectral characteristics of the absorption, fluorescence and RRS, the optimum conditions of the reactions and the properties of the analytical chemistry were investigated. The methods have been successfully applied to determination of some fluoroquinolone antibiotics in human urine samples and tablets. Taking CIP-Ery system as an example, the charge distribution, the enthalpy of formation and the mean polarizability were calculated by density function theory (DFT) method. In addition, the reasons for the enhancement of scattering spectra were discussed.

  9. Time-Average Molecular Rayleigh Scattering Technique for Measurement of Velocity, Denisty, Temperature, and Turbulence Intensity in High Speed Nozzle Flows

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Seasholtz, Richard G.; Elam, Kristie A.; Panda, Jayanta

    2004-01-01

    A molecular Rayleigh scattering based flow diagnostic is developed to measure time average velocity, density, temperature, and turbulence intensity in a 25.4-mm diameter nozzle free jet facility. The spectrum of the Rayleigh scattered light is analyzed using a Fabry-Perot interferometer operated in the static imaging mode. The resulting fringe pattern containing spectral information of the scattered light is recorded using a low noise CCD camera. Nonlinear least squares analysis of the fringe pattern using a kinetic theory model of the Rayleigh scattered light provides estimates of density, velocity, temperature, and turbulence intensity of the gas flow. Resulting flow parameter estimates are presented for an axial scan of subsonic flow at Mach 0.95 for comparison with previously acquired pitot tube data, and axial scans of supersonic flow in an underexpanded screeching jet. The issues related to obtaining accurate turbulence intensity measurements using this technique are discussed.

  10. One centimeter spatial resolution temperature measurements in a nuclear reactor using Rayleigh scatter in optical fiber

    NASA Astrophysics Data System (ADS)

    Sang, A. K.; Gifford, D. K.; Dickerson, B. D.; Fielder, B. F.; Froggatt, M. E.

    2007-07-01

    We present the use of swept wavelength interferometry for distributed fiber-optic temperature measurements in a Nuclear Reactor. The sensors consisted of 2 m segments of commercially available, single mode optical fibers. The interrogation technique is based on measuring the spectral shift of the intrinsic Rayleigh backscatter signal along the optical fiber and converting the spectral shift to temperature.

  11. Impact of Rayleigh backscattering on Stimulated Brillouin Scattering threshold evaluation for 10 Gb/s NRZ-OOK signals.

    PubMed

    Ferrario, M; Marazzi, Lucia; Boffi, Pierpaolo; Righetti, Aldo; Martinelli, Mario

    2009-09-28

    At bit rates comparable with the Brillouin shift, i.e. higher than 10 Gbit/s, the signal and the Brillouin backscattered spectra partially overlap. This implies an interaction between different scattering phenomena occurring through out the optical fiber. In particular we believe that an evaluation of how Rayleigh backscattered components of the modulated signal are subjected to Stokes gain is required. This interaction may lead to an increased backscattered power, which in turn will affect Brillouin threshold estimation. We experimentally verified a decrease of Stimulated Brillouin Scattering (SBS) threshold for 10 Gb/s NRZ-OOK signals with respect to theoretical predictions. Simulations carried out with a numerical model of SBS, accounting for Rayleigh contributions, well predict measured backscattered power levels. On the other hand we also experimentally verified that this SBS threshold decrease does not degrade transmission system performance. Indeed, measured BER curves put into evidence a penalty reduction for signal powers just before the saturation regime, which should be usefully taken into consideration in optical systems power budget planning.

  12. New technique for retrieval of atmospheric temperature profiles from Rayleigh-scatter lidar measurements using nonlinear inversion.

    PubMed

    Khanna, Jaya; Bandoro, Justin; Sica, R J; McElroy, C Thomas

    2012-11-20

    The conventional method of calculating atmospheric temperature profiles using Rayleigh-scattering lidar measurements has limitations that necessitate abandoning temperatures retrieved at the greatest heights, due to the assumption of a pressure value required to initialize the integration at the highest altitude. An inversion approach is used to develop an alternative way of retrieving nightly atmospheric temperature profiles from the lidar measurements. Measurements obtained by the Purple Crow lidar facility located near The University of Western Ontario are used to develop and test this new technique. Our results show temperatures can be reliably retrieved at all heights where measurements with adequate signal-to-noise ratio exist. A Monte Carlo technique was developed to provide accurate estimates of both the systematic and random uncertainties for the retrieved nightly average temperature profile. An advantage of this new method is the ability to seed the temperature integration from the lowest rather than the greatest height, where the variability of the pressure is smaller than in the mesosphere or lower thermosphere and may in practice be routinely measured by a radiosonde, rather than requiring a rocket or satellite-borne measurement. Thus, this new technique extends the altitude range of existing Rayleigh-scatter lidars 10-15 km, producing the equivalent of four times the power-aperture product.

  13. Comprehensive model for studying noise induced by self-homodyne detection of backward Rayleigh scattering in optical fibers.

    PubMed

    Fleyer, Michael; Cahill, James P; Horowitz, Moshe; Menyuk, Curtis R; Okusaga, Olukayode

    2015-10-05

    Backward Rayleigh scattering in optical fibers due to the fluctuations that are "frozen-in" to the fiber during the manufacturing process may limit the performance of optical sensors and bidirectional coherent optical communication systems. In this manuscript we describe a comprehensive model for studying intensity noise induced by spontaneous Rayleigh backscattering in optical systems that are based on self-homodyne detection. Our model includes amplitude and frequency noise of the laser source, random distribution of the scatterers along the fiber, and phase noise induced in fibers due to thermal and mechanical fluctuations. The model shows that at frequencies above about 10 kHz the noise spectrum is determined by the laser white frequency noise. The laser flicker frequency noise becomes the dominant effect at lower frequencies. The noise amplitude depends on the laser polarization. A very good agreement between theory and experiment is obtained for fibers with a length between 500 m to 100 km and for a laser with a linewidth below 5 kHz.

  14. Resonance Rayleigh scattering and resonance non-linear scattering method for the determination of aminoglycoside antibiotics with water solubility CdS quantum dots as probe.

    PubMed

    Liu, Zhengwen; Liu, Shaopu; Wang, Lei; Peng, Juanjuan; He, Youqiu

    2009-09-15

    In pH 6.6 Britton-Robinson buffer medium, the CdS quantum dots capped by thioglycolic acid could react with aminoglycoside (AGs) antibiotics such as neomycin sulfate (NEO) and streptomycin sulfate (STP) to form the large aggregates by virtue of electrostatic attraction and the hydrophobic force, which resulted in a great enhancement of resonance Rayleigh scattering (RRS) and resonance non-linear scattering such as second-order scattering (SOS) and frequency doubling scattering (FDS). The maximum scattering peak was located at 310 nm for RRS, 568 nm for SOS and 390 nm for FDS, respectively. The enhancements of scattering intensity (DeltaI) were directly proportional to the concentration of AGs in a certain ranges. A new method for the determination of trace NEO and STP using CdS quantum dots probe was developed. The detection limits (3 sigma) were 1.7 ng mL(-1) (NEO) and 4.4 ng mL(-1) (STP) by RRS method, were 5.2 ng mL(-1) (NEO) and 20.9 ng mL(-1) (STP) by SOS method and were 4.4 ng mL(-1) (NEO) and 25.7 ng mL(-1) (STP) by FDS method, respectively. The sensitivity of RRS method was the highest. The optimum conditions and influence factors were investigated. In addition, the reaction mechanism was discussed.

  15. The fluorescence and resonance Rayleigh scattering spectral study and analytical application of cerium (IV) and cefoperazone system.

    PubMed

    Yuan, Yusheng; Fu, Shenghui; Xu, Qianying; Yang, Jidong; Hu, Xiaoli; Liu, Shaopu

    2016-06-05

    In weak acidic medium of pH3.5-5.6, Ce(IV) can be reduced by cefoperazone (CPZ) to be Ce(III), which further combined with CPZ to form complex Ce(OH)3CPZ. This complex not only has higher fluorescence than Ce(III), but also results in significant increase of resonance Rayleigh scattering (RRS), second order scattering (SOS) and frequency doubling scattering (FDS). The wavelengths of maximum fluorescence exciting and emission are located at 356 nm/349 nm, while the maximum wavelengths of RRS, SOS and FDS are at 312 nm, 550 nm and 390 nm, respectively. The intensity of fluorescence and scattering are all linear with the concentration of CPZ in certain conditions. The detection limit of most sensitive RRS method for CPZ is 2.1 ng mL(-1). The optimum conditions for detecting CPZ using RRS method are investigated. The effect of co-existing substances shows that the method has excellent selectivity, especially since other cephalosporins don't have similar reactions. Therefore, it can be achieved to determine CPZ in cephalosporins selectively. The paper also focuses on the reaction mechanism, the consistent and contracture of the resultant. The reasons for enhanced intensity are presumed in the meantime.

  16. A rapid and sensitive resonance Rayleigh scattering spectra method for the determination of quinolones in human urine and pharmaceutical preparation.

    PubMed

    Qiao, Man; Wang, Yaqiong; Liu, Shaopu; Liu, Zhongfang; Yang, Jidong; Zhu, Jinghui; Hu, Xiaoli

    2015-03-01

    A new method based on resonance Rayleigh scattering (RRS) was proposed for the determination of quinolones (QNS) at the nanogram level. In pH 3.3-4.4 Britton-Robinson buffer medium, quinolones such as ciprofloxacin, pipemidic acid (PIP), lomefloxacin (LOM), norfloxacin (NOR) and sarafloxacin (SAR) were protonated and reacted with methyl orange (MO) to form an ion-pair complex, which then further formed a six-membered ring chelate with Pd(II). As a result, new RRS spectra appeared and the RRS intensities were enhanced greatly. RRS spectral characteristics of the MO-QNS-Pd(II) systems, the optimum conditions for the reaction, and the influencing factors were investigated. Under optimum conditions, the scattering intensity (∆I) increments were directly proportional to the concentration of QNS with in certain ranges. The method had high sensitivity, and the detection limits (3σ) ranged from 6.8 to 12.6 ng/mL. The proposed method had been successfully applied for the determination of QNS in pharmaceutical formulations and human urine samples. In addition, the mechanism of the reaction system was discussed based on IR, absorption and fluorescence spectral studies. The reasons for the enhancement of scattering spectra were discussed in terms of fluorescence-scattering resonance energy transfer, hydrophobicity and molecular size.

  17. Ultraviolet Rayleigh-Mie lidar with Mie-scattering correction by Fabry-Perot etalons for temperature profiling of the troposphere.

    PubMed

    Hua, Dengxin; Uchida, Masaru; Kobayashi, Takao

    2005-03-01

    A Rayleigh-Mie-scattering lidar system at an eye-safe 355-nm ultraviolet wavelength that is based on a high-spectral-resolution lidar technique is demonstrated for measuring the vertical temperature profile of the troposphere. Two Rayleigh signals, which determine the atmospheric temperature, are filtered with two Fabry-Perot etalon filters. The filters are located on the same side of the wings of the Rayleigh-scattering spectrum and are optically constructed with a dual-pass optical layout. This configuration achieves a high rejection rate for Mie scattering and reasonable transmission for Rayleigh scattering. The Mie signal is detected with a third Fabry-Perot etalon filter, which is centered at the laser frequency. The filter parameters were optimized by numerical calculation; the results showed a Mie rejection of approximately -45 dB, and Rayleigh transmittance greater than 1% could be achieved for the two Rayleigh channels. A Mie correction method is demonstrated that uses an independent measure of the aerosol scattering to correct the temperature measurements that have been influenced by the aerosols and clouds. Simulations and preliminary experiments have demonstrated that the performance of the dual-pass etalon and Mie correction method is highly effective in practical applications. Simulation results have shown that the temperature errors that are due to noise are less than 1 K up to a height of 4 km for daytime measurement for 300 W m(-2) sr(-1) microm(-1) sky brightness with a lidar system that uses 200 mJ of laser energy, a 3.5-min integration time, and a 25-cm telescope.

  18. Study on the interaction between ligustrazine and 12-tungstophosphoric acid using resonance Rayleigh scattering and resonance nonlinear scattering spectra, and its analytical applications.

    PubMed

    Li, Junbo; Yang, Xiaoli; Yang, Jinxiang; Lai, Lina

    2015-08-01

    In an HCl medium (pH 1.5), ligustrazine (2,3,5,6-tetramethylpyrazine, TMP) reacted with 12-tungstophosphoric acid (TP) to form a 3 : 1 ion-association complex. As a result, the intensities of resonance Rayleigh scattering (RRS), second-order scattering (SOS) and frequency doubling scattering (FDS) were greatly enhanced and new scattering spectra appeared. The maximum RRS, SOS and FDS wavelengths of the ion-association complexes were located at 379, 738 and 395 nm, respectively. The scattering intensity increments (ΔIRRS , ΔISOS and ΔIFDS ) were directly proportional to the concentration of ligustrazine within certain ranges. The detection limits (3σ) of RRS, SOS and FDS were 1.6, 3.2 and 2.8 ng/mL. Optimal conditions for the RRS method and factors influencing the method were discussed, and the structure of the ion-association complex and the reaction mechanism were investigated. Transmission electron microscopy (TEM) was used to characterize the structures of the ion-association complex. Based on the ion-association reaction and its spectral response, a rapid, simple and sensitive RRS method for the determination of TMP was developed. It was applied to the determination of TMP in tablet and urine samples with satisfactory results.

  19. Single scattering solution for radiative transfer through Rayleigh and aerosol atmosphere

    NASA Technical Reports Server (NTRS)

    Otterman, J.

    1977-01-01

    A solution is presented to the radiative transfer of the solar irradiation through a turbid atmosphere, based on the single-scattering approximation, i.e., an assumption that a photon that underwent scattering either leaves the top of the atmosphere or strikes the surface. The solution depends on a special idealization of the scattering phase function of the aerosols. The equations developed are subsequently applied to analyze quantitatively the enhancement of the surface irradiation and the enhancement of the scattered radiant emittance as seen from above the atmosphere, caused by the surface reflectance and atmospheric back scattering. An order of magnitude error analysis is presented.

  20. Planar Rayleigh scattering and laser-induced fluorescence for visualization of a hot, Mach 2 annular air jet

    NASA Technical Reports Server (NTRS)

    Balla, R. Jeffrey

    1994-01-01

    Planar Rayleigh scattering (PRS) and planar laser-induced fluorescence (PLIF) were used to investigate the vitiated air component of a coaxial hydrogen/vitiated air nonpremixed turbulent jet flame that is ejected at a Mach number of 2. All experiments were performed with a xenon chloride tunable excimer laser. Planar information for both techniques was obtained using laser sheets 6 cm high, 5 cm wide, and 300 micron thick. In this flow field, the effective Rayleigh cross section of the components in the vitiated air was assumed to be independent of composition. Therefore, the PRS technique produced signals which were proportional to total density. When the flow field was assumed to be at a known and uniform pressure, the PRS signal data for the vitiated air could be converted to temperature information. Also, PLIF images were generated by probing the OH molecule. These images contain striation patterns attributed to small localized instantaneous temperature nonuniformities. The results from the PLIF and PRS techniques were used to show that this flow field contains a nongaseous component, most likely liquid water that can be reduced by increasing the settling chamber wall temperature.

  1. Raman fiber lasers with a random distributed feedback based on Rayleigh scattering

    SciTech Connect

    Churkin, D. V.; Babin, S. A.; Kablukov, S. I.; Podivilov, E. V.; El-Taher, A. E.; Harper, P.; Karalekas, V.; Turitsyn, S. K.; Ania-Castanon, J. D.

    2010-09-15

    We demonstrate lasing based on a random distributed feedback due to the Raman amplified Rayleigh backscattering in different types of cavities with and without conventional point-action reflectors. Quasistationary generation of a narrowband spectrum is achieved despite the random nature of the feedback. The generated spectrum is localized at the reflection or gain spectral maxima in schemes with and without point reflectors, respectively. The length limit for a conventional cavity and the minimal pump power required for the lasing based purely on a random distributed feedback are determined.

  2. Study on erythrosine-phen-Cd(II) systems by resonance Rayleigh scattering, absorption spectra and their analytical applications.

    PubMed

    Tian, Jing; Zhang, Qiqi; Liu, Shaopu; Yang, Jidong; Teng, Ping; Zhu, Jinghui; Qiao, Man; Shi, Ying; Duan, Ruilin; Hu, Xiaoli

    2015-04-05

    In pH 7.0-8.0 KH2PO4-Na2HPO4 buffer solution, Cd(II) reacted with 1,10-phenanthroline to form chelate cation [Cd(phen)3]2+, which further reacted with anion of erythrosine to form ternary ion-association complex through electrostatic attraction and hydrophobic effect. This process could result in remarkable absorption spectra change and produce obvious fading reaction at 528 nm. Absorbance change (ΔA) of system was directly proportional to the concentration of Cd(II). Hereby, a highly sensitive spectrophotometric method for the determination of Cd(II) was established. The molar absorption coefficient was 2.29×10(5) L mol(-1) cm(-1) and the detection limit of Cd(II) was 26.5 ng mL(-1). Furthermore, the resonance Rayleigh scattering (RRS) of this system with two peaks located at 371 and 590 nm enhanced significantly, and second-order scattering (SOS) and frequence doubling scattering (FDS) of this system changed notably at 640 and 350 nm, respectively. Under the optimum conditions, the scattering intensities (ΔIRRS, ΔIDWO-RRS, ΔISOS and ΔIFDS) had good linear relationship with the concentration of Cd(II) in certain ranges. The detection limits of Cd(II) were 1.27 ng mL(-1), 1.39 ng mL(-1), 4.03 ng mL(-1), 5.92 ng mL(-1) and 14.7 ng mL(-1) for dual-wavelength overlapping resonance Rayleigh scattering (DWO-RRS), RRS (371 nm), RRS (590 nm), SOS and FDS, respectively. In addition, the suitable reaction conditions and effects of coexisting substances were investigated. The methods had been successfully applied to the determination of Cd(II) in environmental water samples. The recovery range was between 93.0% and 103.0% and the relative standard deviation (RSD) was between 2.5% and 4.3%. The results were in agreement with those obtained from atomic absorption spectroscopy.

  3. Study on erythrosine-phen-Cd(II) systems by resonance Rayleigh scattering, absorption spectra and their analytical applications

    NASA Astrophysics Data System (ADS)

    Tian, Jing; Zhang, Qiqi; Liu, Shaopu; Yang, Jidong; Teng, Ping; Zhu, Jinghui; Qiao, Man; Shi, Ying; Duan, Ruilin; Hu, Xiaoli

    2015-04-01

    In pH 7.0-8.0 KH2PO4-Na2HPO4 buffer solution, Cd(II) reacted with 1,10-phenanthroline to form chelate cation [Cd(phen)3]2+, which further reacted with anion of erythrosine to form ternary ion-association complex through electrostatic attraction and hydrophobic effect. This process could result in remarkable absorption spectra change and produce obvious fading reaction at 528 nm. Absorbance change (ΔA) of system was directly proportional to the concentration of Cd(II). Hereby, a highly sensitive spectrophotometric method for the determination of Cd(II) was established. The molar absorption coefficient was 2.29 × 105 L mol-1 cm-1 and the detection limit of Cd(II) was 26.5 ng mL-1. Furthermore, the resonance Rayleigh scattering (RRS) of this system with two peaks located at 371 and 590 nm enhanced significantly, and second-order scattering (SOS) and frequence doubling scattering (FDS) of this system changed notably at 640 and 350 nm, respectively. Under the optimum conditions, the scattering intensities (ΔIRRS, ΔIDWO-RRS, ΔISOS and ΔIFDS) had good linear relationship with the concentration of Cd(II) in certain ranges. The detection limits of Cd(II) were 1.27 ng mL-1, 1.39 ng mL-1, 4.03 ng mL-1, 5.92 ng mL-1 and 14.7 ng mL-1 for dual-wavelength overlapping resonance Rayleigh scattering (DWO-RRS), RRS (371 nm), RRS (590 nm), SOS and FDS, respectively. In addition, the suitable reaction conditions and effects of coexisting substances were investigated. The methods had been successfully applied to the determination of Cd(II) in environmental water samples. The recovery range was between 93.0% and 103.0% and the relative standard deviation (RSD) was between 2.5% and 4.3%. The results were in agreement with those obtained from atomic absorption spectroscopy.

  4. Simultaneous measurement of electron and heavy particle temperatures in He laser-induced plasma by Thomson and Rayleigh scattering

    SciTech Connect

    Dzierzega, K.; Mendys, A.; Zawadzki, W.; Pokrzywka, B.; Pellerin, S.

    2013-04-01

    Thomson and Rayleigh scattering methods were applied to quantify the electron and heavy particle temperatures, as well as electron number density, in a laser spark in helium at atmospheric pressure. Plasma was created using 4.5 ns, 25 mJ pulses from Nd:YAG laser at 532 nm. Measurements, performed for the time interval between 20 ns and 800 ns after breakdown, show electron density and temperature to decrease from 7.8 Multiplication-Sign 10{sup 23} m{sup -3} to 2.6 Multiplication-Sign 10{sup 22} m{sup -3} and from 95 900 K to 10 350 K, respectively. At the same time, the heavy particle temperature drops from only 47 000 K down to 4100 K which indicates a two temperature plasma out of local isothermal equilibrium.

  5. Determination of proteins at nanogram levels based on their enhancement effects of Rayleigh light scattering on dibromomethylchlorophosphonazo

    NASA Astrophysics Data System (ADS)

    Li, Qianfeng; Zhang, Hongyi; Xue, Chunxia; Chen, Xingguo; Hu, Zhide

    2000-11-01

    A new Rayleigh light scattering (RLS) assay of protein was conducted in this paper. At the optimum pH conditions, and in the presence of Tween-20, the weak RLS of dibromomethylchlorophosphonazo (DBM-CPA) can be enhanced greatly by the addition of proteins. Based on this, the reactions of DBM-CPA and proteins were studied. A new quantitative determination method for proteins has been developed. The method is simple, practical and relatively free from interference from coexisting substances, as well as much more sensitive (the dynamic ranges of 0.065-40.05 μg ml -1 and detection limit of 30 ng ml -1 for bovine serum albumin (BSA)) than most of the existing assays. The determination results of human body serum samples are identical to those by the CBB method, with relative S.D. of six determination of 0.5-2.2%.

  6. A sensitive and selective resonance Rayleigh scattering method for quick detection of avidin using affinity labeling Au nanoparticles

    NASA Astrophysics Data System (ADS)

    Wang, Qi; Huang, Xi; Fu, Xuan; Deng, Huan; Ma, Meihu; Cai, Zhaoxia

    2016-06-01

    Avidin is a glycoprotein with antinutritional property, which should be limited in daily food. We developed an affinity biosensor system based on resonance Rayleigh scattering (RRS) and using affinity biotin labeling Au nanoparticles (AuNPs). This method was selective and sensitive for quick avidin detection due to the avidin-biotin affinitive interaction. Under optimal conditions, RRS intensity of biotin-AuNPs increase linearly with an increasing concentration of avidin from 5 to 160 ng/mL. The lower limit of detection was 0.59 ng/mL. This rapid and selective avidin detection method was used in synthetic samples and egg products with recoveries of between 102.97 and 107.92%, thereby demonstrating the feasible and practical application of this assay.

  7. A sensitive and selective resonance Rayleigh scattering method for quick detection of avidin using affinity labeling Au nanoparticles.

    PubMed

    Wang, Qi; Huang, Xi; Fu, Xuan; Deng, Huan; Ma, Meihu; Cai, Zhaoxia

    2016-06-05

    Avidin is a glycoprotein with antinutritional property, which should be limited in daily food. We developed an affinity biosensor system based on resonance Rayleigh scattering (RRS) and using affinity biotin labeling Au nanoparticles (AuNPs). This method was selective and sensitive for quick avidin detection due to the avidin-biotin affinitive interaction. Under optimal conditions, RRS intensity of biotin-AuNPs increase linearly with an increasing concentration of avidin from 5 to 160 ng/mL. The lower limit of detection was 0.59 ng/mL. This rapid and selective avidin detection method was used in synthetic samples and egg products with recoveries of between 102.97 and 107.92%, thereby demonstrating the feasible and practical application of this assay.

  8. Light scattering by tenuous particles - A generalization of the Rayleigh-Gans-Rocard approach

    NASA Technical Reports Server (NTRS)

    Acquista, C.

    1976-01-01

    We consider scattering by arbitrarily shaped particles that satisfy two conditions: (1) that the polarizability of the particle relative to the ambient medium be small compared to 1 and (2) that the phase shift introduced by the particle be less than 2. We solve the integro-differential equation proposed by Shifrin by using the method of successive iterations and then applying a Fourier transform. For the second iteration, results are presented that accurately describe scattering by a broad class of particles. The phase function and other elements of the scattering matrix are shown to be in excellent agreement with Mie theory for spherical scatterers.

  9. On-Resonance Fluorescence, Resonance Rayleigh Scattering, and Ratiometric Resonance Synchronous Spectroscopy of Molecular- and Quantum Dot-Fluorophores.

    PubMed

    Siriwardana, Kumudu; Nettles, Charles B; Vithanage, Buddhini C N; Zhou, Yadong; Zou, Shengli; Zhang, Dongmao

    2016-09-20

    Existing studies on molecular fluorescence have almost exclusively been focused on Stokes-shifted fluorescence spectroscopy (SSF) in which the emitted photon is detected at the wavelengths longer than that for the excitation photons. Information on fluorophore on-resonance fluorescence (ORF) and resonance Rayleigh scattering (RRS) is limited and often problematic due to the complex interplay of the fluorophore photon absorption, ORF emission, RRS, and solvent Rayleigh scattering. Reported herein is a relatively large-scale systematic study on fluorophore ORF and RRS using the conventional UV-vis extinction and SSF measurements in combination with the recently reported ratiometric resonance synchronous spectroscopic (R2S2, pronounced as "R-Two-S-Two") method. A series of fundamental parameters including fluorophore ORF cross sections and quantum yields have been quantified for the first time for a total of 12 molecular and 6 semiconductor quantum dot (QD) fluorophores. All fluorophore spectra comprise a well-defined Gaussian peak with a full width at half-maximum ranging from 4 to 30 nm. However, the RRS features of fluorophores differ drastically. The effect of fluorophore aggregation on its RRS, UV-vis, R2S2, and SSF spectra was also discussed. This work highlights the critical importance of the combined UV-vis extinction, SSF, and R2S2 spectroscopic measurements for material characterizations. The method and insights described in this work can be directly used for improving the reliability of RRS spectroscopic methods in chemical analysis. In addition, it should pave the way for developing novel R2S2-based analytical applications.

  10. Flat amplitude multiwavelength Brillouin-Raman comb fiber laser in Rayleigh-scattering-enhanced linear cavity.

    PubMed

    Zamzuri, A K; Mahdi, M A; Ahmad, A; Md Ali, M I; Al-Mansoori, M H

    2007-03-19

    We investigate the amplitude flatness of Rayleigh-assisted Brillouin-Raman comb laser in a linear cavity in which feedbacks are formed by high-reflectivity mirror. The optimization of Brillouin pump power and wavelength is very crucial in order to obtain a uniform power level between Stokes lines. The Brillouin pump must have a relatively large power and its wavelength must be located closer to the Raman peak gain region. The flat-amplitude bandwidth is also determined by the choice of Raman pump wavelengths. A flat-amplitude bandwidth of 30.7 nm from 1527.32 to 1558.02 nm is measured when Raman pump wavelengths are set to 1435 and 1450 nm. 357 uniform Brillouin Stokes lines with 0.086 nm spacing are generated across the wavelength range. The average signal-to-noise ratio of 17 dB is obtained for all the Brillouin Stokes lines.

  11. Distributed Temperature and Strain Discrimination with Stimulated Brillouin Scattering and Rayleigh Backscatter in an Optical Fiber

    PubMed Central

    Zhou, Da-Peng; Li, Wenhai; Chen, Liang; Bao, Xiaoyi

    2013-01-01

    A distributed optical fiber sensor with the capability of simultaneously measuring temperature and strain is proposed using a large effective area non-zero dispersion shifted fiber (LEAF) with sub-meter spatial resolution. The Brillouin frequency shift is measured using Brillouin optical time-domain analysis (BOTDA) with differential pulse-width pair technique, while the spectrum shift of the Rayleigh backscatter is measured using optical frequency-domain reflectometry (OFDR). These shifts are the functions of both temperature and strain, and can be used as two independent parameters for the discrimination of temperature and strain. A 92 m measurable range with the spatial resolution of 50 cm is demonstrated experimentally, and accuracies of ±1.2 °C in temperature and ±15 με in strain could be achieved. PMID:23385406

  12. Distributed temperature and strain discrimination with stimulated brillouin scattering and rayleigh backscatter in an optical fiber.

    PubMed

    Zhou, Da-Peng; Li, Wenhai; Chen, Liang; Bao, Xiaoyi

    2013-01-31

    A distributed optical fiber sensor with the capability of simultaneously measuring temperature and strain is proposed using a large effective area non-zero dispersion shifted fiber (LEAF) with sub-meter spatial resolution. The Brillouin frequency shift is measured using Brillouin optical time-domain analysis (BOTDA) with differential pulse-width pair technique, while the spectrum shift of the Rayleigh backscatter is measured using optical frequency-domain reflectometry (OFDR). These shifts are the functions of both temperature and strain, and can be used as two independent parameters for the discrimination of temperature and strain. A 92 m measurable range with the spatial resolution of 50 cm is demonstrated experimentally, and accuracies of ±1.2 °C in temperature and ±15 με in strain could be achieved.

  13. Near-Field Nanofluid Concentration Measurement by Rayleigh Particle Scattering Bragg Grating Evanescent Wave

    NASA Astrophysics Data System (ADS)

    Huang, Xue-Feng; Li, Sheng-Ji

    2014-04-01

    We report an approach to detect near-field nanofluid concentration by scattering Bragg grating evanescent wave (EW). Since the suspended nanoparticles can enhance the scattering intensity of the EW from the thinned and tapered fiber with Bragg grating, the reflectance ratio of Bragg grating is dependent on the corresponding refractive index (RI) of the nanofluid at different nanoparticle volume fraction. A critical reflectance ratio measurement identifies the nanofluid concentration. Theory and simulation of scattering Bragg grating EW was analyzed. The scattering Bragg grating EW fiber sensing probe was designed and fabricated by the wet chemical etching method, and calibration was made by several chemical solutions without suspended nanoparticles. The example application of the nanofluid containing dispersed 40 nm SiO2 nanoparticles demonstrates the feasibility. The reflectance ratio decreases by over 3.2% with the nanofluid concentration increasing from 0.25 wt.% to 4 wt.%, while the temperature disturbance can be negligible.

  14. Resonance Rayleigh scattering, frequency doubling scattering and absorption spectrum of the interaction for mebendazole with 12-tungstophosphoric acid and its analytical applications.

    PubMed

    Tian, Fengling; Yang, Jidong; Huang, Wei; Zhou, Shang; Yao, Gengyang

    2013-12-01

    The interaction of mebendazole (MBZ) with 12-tungstophosphoric acid (TP) has been investigated by using resonance Rayleigh scattering (RRS) and frequency doubling scattering (FDS) combining with absorption spectrum. In pH 1.0 HCl medium, MBZ reacted with TP to form 3:1 ion-association complex. As a result, not only the spectrum of absorption was changed, but also the intensities of RRS and FDS were enhanced greatly. The maximum RRS, FDS and absorption wavelengths are located at 372, 392 and 260 nm, respectively. The increments of scattering intensity (ΔI) and absorption (ΔA) are directly proportional to the concentrations of MBZ in certain ranges. The detection limits (3σ) of RRS, FDS and absorption are 0.56, 0.86 and 130.16 ng/mL, respectively. The sensitivity of RRS method is higher than FDS and absorption methods. The optimum conditions of RRS method and the influence factors were discussed in the paper, in addition, the structure of ion-association complex and the reaction mechanism were investigated. Based on the ion-association reaction and its spectral response, the rapid, simple and sensitive RRS method for the determination of MBZ has been developed.

  15. Structure of the pyridine-chloranil complex in solution: a surprise from depolarized hyper-Rayleigh scattering measurements.

    PubMed

    Pandey, Ravindra; Mukhopadhyay, S; Ramasesha, S; Das, Puspendu K

    2011-12-01

    In this article, we report the structure of a 1:1 charge transfer complex between pyridine (PYR) and chloranil (CHL) in solution (CHCl(3)) from the measurement of hyperpolarizability (β(HRS)) and linear and circular depolarization ratios, D and D', respectively, by the hyper-Rayleigh scattering technique and state-of-the-art quantum chemical calculations. Using linearly (electric field vector along X) and circularly polarized incident light, respectively, we have measured two macroscopic depolarization ratios D = I(X,X)(2ω)/I(X,Z)(2ω) and D' = I(X,C)(2ω)/I(Z,C)(2ω) in the laboratory fixed XYZ frame by detecting the second harmonic (SH) scattered light in a polarization resolved fashion. The stabilization energy and the optical gap calculated through the MP2/cc-pVDZ method using Gaussian09 were not significantly different to distinguish between the cofacial and T-shape structures. Only when the experimentally obtained β(HRS) and the depolarization ratios, D and D', were matched with the theoretically computed values from single and double configuration interaction (SDCI) calculations performed using the ZINDO-SCRF technique, we concluded that the room temperature equilibrium structure of the complex is cofacial. This is in sharp contrast to an earlier theoretical prediction of the T-shape structure of the complex.

  16. Double-wavelength overlapping resonance Rayleigh scattering technique for the simultaneous quantitative analysis of three β-adrenergic blockade

    NASA Astrophysics Data System (ADS)

    Tan, Xuanping; Yang, Jidong; Li, Qin; Yang, Qiong; Shen, Yizhong

    2016-05-01

    Four simple and accurate spectrophotometric methods were proposed for the simultaneous determination of three β-adrenergic blockade, e.g. atenolol, metoprolol and propranolol. The methods were based on the reaction of the three drugs with erythrosine B (EB) in a Britton-Robinson buffer solution at pH 4.6. EB could combine with the drugs to form three ion-association complexes, which resulted in the resonance Rayleigh scattering (RRS) intensity that is enhanced significantly with new RRS peaks that appeared at 337 nm and 370 nm, respectively. In addition, the fluorescence intensity of EB was also quenched. The enhanced scattering intensities of the two peaks and the fluorescence quenched intensity of EB were proportional to the concentrations of the drugs, respectively. What is more, the RRS intensity overlapped with the double-wavelength of 337 nm and 370 nm (so short for DW-RRS) was also proportional to the drugs concentrations. So, a new method with highly sensitive for simultaneous determination of three bisoprolol drugs was established. Finally, the optimum reaction conditions, influencing factors and spectral enhanced mechanism were investigated. The new DW-RRS method has been applied to simultaneously detect the three β-blockers in fresh serum with satisfactory results.

  17. Quantitative fuel vapor/air mixing imaging in droplet/gas regions of an evaporating spray flow using filtered Rayleigh scattering.

    PubMed

    Allison, Patton M; McManus, Thomas A; Sutton, Jeffrey A

    2016-03-15

    This Letter demonstrates the application of filtered Rayleigh scattering (FRS) for quantitative two-dimensional fuel vapor/air mixing measurements in an evaporating hydrocarbon fuel spray flow. Using the FRS approach, gas-phase measurements are made in the presence of liquid-phase droplets without interference. Effective suppression of the liquid-phase droplet scattering using FRS is enabled by the high spectral purity of the current Nd:YAG laser system. Simultaneous Mie-scattering imaging is used to visualize the droplet field and illustrate the droplet loading under which the FRS imaging is applied in the current spray flows. The initial quantification of the FRS imaging is based on calibration measurements from a flow cell of known fuel vapor/air mixtures, while future work targets the utilization of a Rayleigh-Brillouin spectral model for quantification of the FRS signals.

  18. Dense medium radiative transfer theory for two scattering layers with a Rayleigh distribution of particle sizes

    SciTech Connect

    West, R.; Tsang, Leung; Winebrenner, D.P. )

    1993-03-01

    Dense medium radiative transfer theory is applied to a three-layer model consisting of two scattering layers overlying a homogeneous half space with a size distribution of particles in each layer. A model with a distribution of sizes gives quite different results than those obtained from a model with a single size. The size distribution is especially important in the low frequency limit when scattering is strongly dependent on particle size. The size distribution and absorption characteristics also affect the extinction behavior as a function of fractional volume. Theoretical results are also compared with experimental data. The sizes, permittivities, and densities used in the numerical illustrations are typical values for snow.

  19. LINE-INTERLOCKING EFFECTS ON POLARIZATION IN SPECTRAL LINES BY RAYLEIGH AND RAMAN SCATTERING

    SciTech Connect

    Sampoorna, M.; Nagendra, K. N.; Stenflo, J. O. E-mail: knn@iiap.res.in

    2013-06-20

    The polarized spectrum of the Sun and stars is formed from the scattering of anisotropic radiation on atoms. Interpretation of this spectrum requires the solution of polarized line transfer in multilevel atomic systems. While sophisticated quantum theories of polarized line formation in multilevel atomic systems exist, they are limited by the approximation of complete frequency redistribution in scattering. The partial frequency redistribution (PRD) in line scattering is a necessary component in modeling the polarized spectra of strong lines. The polarized PRD line scattering theories developed so far confine themselves to a two-level or a two-term atom model. In this paper, we present a heuristic approach to the problem of polarized line formation in multilevel atoms taking into account the effects of PRD and a weak magnetic field. Starting from the unpolarized PRD multilevel atom approach of Hubeny et al., we incorporate the polarization state of the radiation field. However, the lower level polarization is neglected. Two iterative methods of solving the polarized PRD line transfer in multilevel atoms are also presented. Taking the example of a five-level Ca II atom model, we present illustrative results for an isothermal one-dimensional model atmosphere.

  20. Confocal detection of Rayleigh scattering for residual stress measurement in chemically tempered glass

    NASA Astrophysics Data System (ADS)

    Hödemann, S.; Möls, P.; Kiisk, V.; Murata, T.; Saar, R.; Kikas, J.

    2015-12-01

    A new optical method is presented for evaluation of the stress profile in chemically tempered (chemically strengthened) glass based on confocal detection of scattered laser beam. Theoretically, a lateral resolution of 0.2 μm and a depth resolution of 0.6 μm could be achieved by using a confocal microscope with high-NA immersion objective. The stress profile in the 250 μm thick surface layer of chemically tempered lithium aluminosilicate glass was measured with a high spatial resolution to illustrate the capability of the method. The confocal method is validated using transmission photoelastic and Na+ ion concentration profile measurement. Compositional influence on the stress-optic coefficient is calculated and discussed. Our method opens up new possibilities for three-dimensional scattered light tomography of mechanical imaging in birefringent materials.

  1. Confocal detection of Rayleigh scattering for residual stress measurement in chemically tempered glass

    SciTech Connect

    Hödemann, S. Möls, P.; Kiisk, V.; Saar, R.; Kikas, J.; Murata, T.

    2015-12-28

    A new optical method is presented for evaluation of the stress profile in chemically tempered (chemically strengthened) glass based on confocal detection of scattered laser beam. Theoretically, a lateral resolution of 0.2 μm and a depth resolution of 0.6 μm could be achieved by using a confocal microscope with high-NA immersion objective. The stress profile in the 250 μm thick surface layer of chemically tempered lithium aluminosilicate glass was measured with a high spatial resolution to illustrate the capability of the method. The confocal method is validated using transmission photoelastic and Na{sup +} ion concentration profile measurement. Compositional influence on the stress-optic coefficient is calculated and discussed. Our method opens up new possibilities for three-dimensional scattered light tomography of mechanical imaging in birefringent materials.

  2. Resonant Rayleigh scattering for the determination of trace amounts of mercury (II) with thiocyanate and basic triphenylmethane dyes

    SciTech Connect

    Liu, S.; Liu, Z.; Zhou, G.

    1998-05-01

    Intense resonance Rayleigh scattering (RRS) appears when mercury (II) reacts with thiocyanate and a basic triphenylmethane dye (BTPMD), such as crystal violet (CV), ethyl violet (EV), brilliant green (BG), malachite green (MG) or indine green (IG), to form an ion-association complex of the type (BTPMD){sub 2}[Hg(SCN){sub 4}]. The characteristics of RRS spectra of the ion-association complexes and suitable conditions for the reactions were investigated. The intensity of RRS is directly proportional to the concentration of mercury (II) in the range of 0--2.0 {micro}g/25 ml. The RRS methods have very high sensitivities for determination of mercury (II); their detection limits are between 1.68 ng/ml and 6.00 ng/ml on different dye systems. The effects of foreign ions and ways to improve the selectivity were studied. The new highly sensitive methods for the determination of trace amounts of mercury based on the RRS of the ion-association complexes have been developed.

  3. Measurement of time series variation of thermal diffusivity of magnetic fluid under magnetic field by forced Rayleigh scattering method

    NASA Astrophysics Data System (ADS)

    Motozawa, Masaaki; Muraoka, Takashi; Motosuke, Masahiro; Fukuta, Mitsuhiro

    2017-04-01

    It can be expected that the thermal diffusivity of a magnetic fluid varies from time to time after applying a magnetic field because of the growth of the inner structure of a magnetic fluid such as chain-like clusters. In this study, time series variation of the thermal diffusivity of a magnetic fluid caused by applying a magnetic field was investigated experimentally. For the measurement of time series variation of thermal diffusivity, we attempted to apply the forced Rayleigh scattering method (FRSM), which has high temporal and high spatial resolution. We set up an optical system for the FRSM and measured the thermal diffusivity. A magnetic field was applied to a magnetic fluid in parallel and perpendicular to the heat flux direction, and the magnetic field intensity was 70 mT. The FRSM was successfully applied to measurement of the time series variation of the magnetic fluid from applying a magnetic field. The results show that a characteristic configuration in the time series variation of the thermal diffusivity of magnetic fluid was obtained in the case of applying a magnetic field parallel to the heat flux direction. In contrast, in the case of applying a magnetic field perpendicular to the heat flux, the thermal diffusivity of the magnetic fluid hardly changed during measurement.

  4. Semi-classical dynamics of superradiant Rayleigh scattering in a Bose-Einstein condensate

    NASA Astrophysics Data System (ADS)

    Müller, J. H.; Witthaut, D.; le Targat, R.; Arlt, J. J.; Polzik, E. S.; Hilliard, A. J.

    2016-10-01

    Due to its coherence properties and high optical depth, a Bose-Einstein condensate [BEC] provides an ideal setting to investigate collective atom-light interactions. Superradiant light scattering [SLS] in a BEC is a fascinating example of such an interaction. It is an analogous process to Dicke superradiance, in which an electronically inverted sample decays collectively, leading to the emission of one or more light pulses in a well-defined direction. Through time-resolved measurements of the superradiant light pulses emitted by an end-pumped BEC, we study the close connection of SLS with Dicke superradiance. A 1D model of the system yields good agreement with the experimental data and shows that the dynamics result from the structures that build up in the light and matter-wave fields along the BEC. This paves the way for exploiting the atom-photon correlations generated by the superradiance.

  5. Measurement of the depolarization ratio of Rayleigh scattering at absorption bands

    NASA Astrophysics Data System (ADS)

    Anglister, J.; Steinberg, I. Z.

    1981-01-01

    Measurements of the depolarization ratio ρv of light scattered by the pigments lycopene and β-carotene at the red part of their absorption bands yielded values which are very close to the theoretical value 1/3 of a fully anisotropic molecular polarizability, i.e., that due to an electric dipole moment. Measurements of ρv at the blue edge of the visible absorption band of pinacyanol chloride yielded a value of 0.75 at 472.2 nm, which is the maximum value that a depolarization ratio can assume, and is attained if the average molecular polarizability is zero. This is possible only if the diagonalized polarizability tensor has at least one negative element to counterbalance the positive ones. A negative refractive index at the blue edge of the absorption band is thus experimentally demonstrated.

  6. Determination of nucleic acids with tetra-( N-hexadecylpyridiniumyl) porphyrin sensitized by cetyltrimethylammonium bromide (CTMAB) using a Rayleigh light-scattering technique

    NASA Astrophysics Data System (ADS)

    Zhu, Changqing; Zhuo, Shujuan; Li, Yongxin; Wang, Lun; Zhao, Danhua; Chen, Jinlong; Wu, Yuqin

    2004-03-01

    Using a common spectrofluorometer to measure the intensity of Rayleigh light-scattering (RLS), a method for determination of nucleic acids has been developed. At pH 10.24 and ionic strength 0.01 mol l -1 (NaCl), the Rayleigh light-scattering of the tetra-( N-hexadecylpyridiniumyl) porphyrin (TC 16PyP) is greatly enhanced by nucleic acids in the presence of cetyltrimethylammonium bromide (CTMAB), with the scattering peak located at 311.8 nm. The enhanced RLS intensity is in proportion to the concentration of calf thymus DNA (ctDNA) in the range 0.2-6.0 μg ml -1 and to that of fish sperm DNA (fsDNA) in the range 0.05-3.0 μg ml -1. The limits of detection are 0.016 μg ml -1 for calf thymus DNA and 0.023 μg ml -1 for fish sperm DNA when the concentration of TPP was chosen 2.0×10 -6 mol l -1. Four synthetic samples were determined satisfactorily.

  7. Development of a Rayleigh Scattering Diagnostic for Time-Resolved Gas Flow Velocity, Temperature, and Density Measurements in Aerodynamic Test Facilities

    NASA Technical Reports Server (NTRS)

    Mielke, Amy F.; Elam, Kristie A.; Sung, Chih-Jen

    2007-01-01

    A molecular Rayleigh scattering technique is developed to measure time-resolved gas velocity, temperature, and density in unseeded turbulent flows at sampling rates up to 32 kHz. A high power continuous-wave laser beam is focused at a point in an air flow field and Rayleigh scattered light is collected and fiber-optically transmitted to the spectral analysis and detection equipment. The spectrum of the light, which contains information about the temperature and velocity of the flow, is analyzed using a Fabry-Perot interferometer. Photomultiplier tubes operated in the photon counting mode allow high frequency sampling of the circular interference pattern to provide time-resolved flow property measurements. An acoustically driven nozzle flow is studied to validate velocity fluctuation measurements, and an asymmetric oscillating counterflow with unequal enthalpies is studied to validate the measurement of temperature fluctuations. Velocity fluctuations are compared with constant temperature anemometry measurements and temperature fluctuations are compared with constant current anemometry measurements at the same locations. Time-series and power spectra of the temperature and velocity measurements are presented. A numerical simulation of the light scattering and detection process was developed and compared with experimental data for future use as an experiment design tool.

  8. Surface roughness considerations for atmospheric correction of ocean color sensors. I - The Rayleigh-scattering component. II - Error in the retrieved water-leaving radiance

    NASA Technical Reports Server (NTRS)

    Gordon, Howard R.; Wang, Menghua

    1992-01-01

    The first step in the Coastal Zone Color Scanner (CZCS) atmospheric-correction algorithm is the computation of the Rayleigh-scattering (RS) contribution, L sub r, to the radiance leaving the top of the atmosphere over the ocean. In the present algorithm, L sub r is computed by assuming that the ocean surface is flat. Calculations of the radiance leaving an RS atmosphere overlying a rough Fresnel-reflecting ocean are presented to evaluate the radiance error caused by the flat-ocean assumption. Simulations are carried out to evaluate the error incurred when the CZCS-type algorithm is applied to a realistic ocean in which the surface is roughened by the wind. In situations where there is no direct sun glitter, it is concluded that the error induced by ignoring the Rayleigh-aerosol interaction is usually larger than that caused by ignoring the surface roughness. This suggests that, in refining algorithms for future sensors, more effort should be focused on dealing with the Rayleigh-aerosol interaction than on the roughness of the sea surface.

  9. Study on interaction between palladium(ІІ)-Linezolid chelate with eosin by resonance Rayleigh scattering, second order of scattering and frequency doubling scattering methods using Taguchi orthogonal array design.

    PubMed

    Thakkar, Disha; Gevriya, Bhavesh; Mashru, R C

    2014-03-25

    Linezolid reacted with palladium to form 1:1 binary cationic chelate which further reacted with eosin dye to form 1:1 ternary ion association complex at pH 4 of Walpole's acetate buffer in the presence of methyl cellulose. As a result not only absorption spectra were changed but Resonance Rayleigh Scattering (RRS), Second-order Scattering (SOS) and Frequency Doubling Scattering (FDS) intensities were greatly enhanced. The analytical wavelengths of RRS, SOS and FDS (λex/λem) of ternary complex were located at 538 nm/538nm, 240 nm/480 nm and 660 nm/330 nm, respectively. The linearity range for RRS, SOS and FDS methods were 0.01-0.5 μg mL(-1), 0.1-2 μg mL(-1) and 0.2-1.8 μg mL(-1), respectively. The sensitivity order of three methods was as RRS>SOS>FDS. Accuracy of all methods were determined by recovery studies and showed recovery between 98% and 102%. Intraday and inter day precision were checked for all methods and %RSD was found to be less than 2 for all methods. The effects of foreign substances were tested on RRS method and it showed the method had good selectivity. For optimization of process parameter, Taguchi orthogonal array design L8(2(4)) was used and ANOVA was adopted to determine the statistically significant control factors that affect the scattering intensities of methods. The reaction mechanism, composition of ternary ion association complex and reasons for scattering intensity enhancement was discussed in this work.

  10. Banquet Speech Some Sketches Of Rayleigh

    NASA Astrophysics Data System (ADS)

    Howard, John N.

    1985-11-01

    Several short sketches are presented of Lord Rayleigh, to show his method of working and his interaction with his fellow scientists. The topics discussed are: his research on the blue of the sky (Rayleigh scattering); his rescue of Waterston from near-oblivion; his research on surface acoustic waves (Rayleigh waves); his collaboration with Agnes Pockels; his research on blackbody radiation (the Rayleigh-Jeans Law).

  11. Incorporation of flow injection analysis with dual-wavelength overlapping resonance Rayleigh scattering for rapid determination of malachite green and its metabolite in fish.

    PubMed

    Zhu, Jinghui; Qin, Mingyou; Liu, Shaopu; Liu, Zhongfang; Yang, Jidong; Hu, Xiaoli

    2014-09-15

    A flow injection analysis (FIA) system combined with dual-wavelength overlapping resonance Rayleigh scattering (DWO-RRS) has been established and validated for rapid determination of malachite green (MG) and its metabolite in fish samples. Under experimental condition, MG would react with Erythrosin (Ery) to form ion-association complexes, resulting in the occurrence of two RRS peaks and a dramatic enhancement of RRS intensity. The maximum RRS peaks were located at 286 nm and 337 nm. It is noted that the increments of both of these two peaks were proportional to the concentration of MG. The detection limit of DWO-RRS was 1.5 ng/mL, which was comparable to several reported methods. Moreover, the results of real sample analysis exhibited an acceptable recovery between 97.5% and 103.6%, indicating that the method had good reproducibility.

  12. Incorporation of flow injection analysis with dual-wavelength overlapping resonance Rayleigh scattering for rapid determination of malachite green and its metabolite in fish

    NASA Astrophysics Data System (ADS)

    Zhu, Jinghui; Qin, Mingyou; Liu, Shaopu; Liu, Zhongfang; Yang, Jidong; Hu, Xiaoli

    2014-09-01

    A flow injection analysis (FIA) system combined with dual-wavelength overlapping resonance Rayleigh scattering (DWO-RRS) has been established and validated for rapid determination of malachite green (MG) and its metabolite in fish samples. Under experimental condition, MG would react with Erythrosin (Ery) to form ion-association complexes, resulting in the occurrence of two RRS peaks and a dramatic enhancement of RRS intensity. The maximum RRS peaks were located at 286 nm and 337 nm. It is noted that the increments of both of these two peaks were proportional to the concentration of MG. The detection limit of DWO-RRS was 1.5 ng/mL, which was comparable to several reported methods. Moreover, the results of real sample analysis exhibited an acceptable recovery between 97.5% and 103.6%, indicating that the method had good reproducibility.

  13. Highly sensitive and selective determination of fluorine ion by graphene oxide/nanogold resonance Rayleigh scattering-energy transfer analytical platform.

    PubMed

    Liang, Aihui; Peng, Jing; Liu, Qingye; Wen, Guiqing; Lu, Zhujun; Jiang, Zhiliang

    2015-08-15

    In pH 4.0 acetate buffer solution, fluorine ions react with fluorine reagent (FR) and La(III) to generate blue ternary complex that exhibited strong absorption at about 370 nm. Upon addition of graphene oxide/nanogold (GO/NG) as resonance Rayleigh scattering (RRS) spectral probe with strong RRS peak at 370 nm, the color changed to gray, and the RRS intensity decreased with the increase of fluorine ion concentration due to the RRS energy transfer (RRSET) from GO/NG to the complex. Under the selected condition, the decreased RRS peak ΔI370 nm was linear to fluorine ion concentration in the range of 6.0 × 10(-8)-1.3 × 10(-5)mol/L, with a detection limit of 3.0 × 10(-8)mol/L F(-). This RRSET method was applied to the analysis of fluorine in toothpaste and water samples, with satisfactory results.

  14. The analytical application and spectral investigation of DNA-CPB-emodin and sensitive determination of DNA by resonance Rayleigh light scattering technique

    NASA Astrophysics Data System (ADS)

    Bi, Shuyun; Wang, Yu; Wang, Tianjiao; Pang, Bo; Zhao, Tingting

    2013-01-01

    A new sensitive DNA probe containing cetylpyridinium bromide (CPB) and emodin (an effective component of Chinese herbal medicine) was developed using the resonance Rayleigh light scattering (RLS) technique. A novel assay was first developed to detect DNA at nanogram level based on the ternary system of DNA-CPB-emodin. The RLS signal of DNA was enhanced remarkably in the presence of emodin-CPB, and the enhanced RLS intensity at 340.0 nm was in direct proportion to DNA concentration in the range of 0.01-2.72 μg mL-1 with a good linear relationship. The detection limit was 1.5 ng mL-1. Three synthetic DNA samples were measured obtaining satisfactory results, the recovery was 97.6-107.3%.

  15. Effects of (R)- and (S)-propranolol hydrochloride enantiomers on the resonance Rayleigh scattering spectra with erythrosine B as probe and their analytical applications.

    PubMed

    Yang, Jidong; Wang, Ernv; Zhou, Shang; Yang, Qiong

    2015-03-01

    Propranolol, a chiral drug with two configurations, i.e., (R)-propranolol hydrochloride (RPH) and (S)-propranolol hydrochloride (SPH), has racemes that can be used in clinical diagnosis due to their synergistic effects. SPH has a β-receptor blocking effect, and RPH has an antiarrhythmic effect. In pH 4.6 Britton-Robinson (BR) buffer solution, both RPH and SPH can react with erythrosine B to form 1:1 ion-association complexes. In the SPH-Ery B reaction system, a remarkable enhancement of the resonance Rayleigh scattering (RRS) signal located at 338 nm was observed. However, a similar phenomenon was not obvious and was unstable in the RPH-Ery B reaction system. Based on this result, a simple, novel and sensitive method for the determination of SPH was proposed based on the RRS technique. The linear range and limit of detection were 0.0680~4.0 µg mL(-1) and 20.6 ng mL(-1), respectively. Additionally, the spectroscopic approaches of frequency doubling scattering (FDS) and second-order scattering (SOS) were also proposed for SPH detection in this article. The interaction information regarding the mechanism of the reaction, suitable reaction conditions, influencing factors and the effects of mixed solutions were our investigation aims. The method had been applied to the determination of SPH in fresh serum and urine samples of healthy human subjects with satisfactory results.

  16. Neutron activation analysis and X-ray Rayleigh and Raman scattering of hair and nail clippings as noninvasive bioindicators for Cu liver status in Labrador Retrievers

    PubMed Central

    Bueno, Maria Izabel Maretti Silveira; Bortoleto, Gisele G.; Hoffmann, Gaby; van den Ingh, Ted S. G. A. M.; Rothuizen, Jan

    2008-01-01

    The heritability of chronic hepatitis in the Labrador Retriever is studied with the aim of identifying the related gene mutation. Identification of cases and controls is largely based on instrumental neutron activation analysis (INAA) Cu determination in liver biopsies. The burden for these companion animals may be reduced if nail clippings and hair (fur) could serve as a noninvasive indicator for the hepatic Cu concentrations. No correlation was found between hepatic Cu concentrations and Cu concentrations in hair and nail samples. However, hair and nail samples were also analyzed by X-ray tube excitation, taking advantage of the X-ray Compton, Rayleigh, and Raman scattering which reflects the organic components such as the type of melanin. Principal component analysis provided first indications that some differentiation between healthy and sick dogs could indeed be obtained from hair and nail analysis. Figure Principal component analysis of scattered region of x-ray fluorescence spectra of Labrador dog nails, demonstrating the differentiation towards dogs with high and low Cu liver levels (respectively positive and negative PC2 values) reflecting hepatitis, as well as gender (PC1: negative values for female and positive values for males) PMID:18264701

  17. Refinement of the Compton-Rayleigh scatter ratio method for use on the Mars Science Laboratory alpha particle X-ray spectrometer: II - Extraction of invisible element content

    NASA Astrophysics Data System (ADS)

    Perrett, Glynis M.; Campbell, John L.; Gellert, Ralf; King, Penelope L.; Nield, Emily; O'Meara, Joanne M.; Pradler, Irina

    2016-02-01

    The intensity ratio C/R between Compton and Rayleigh scatter peaks of the exciting Pu L X-rays in the alpha particle X-ray spectrometer (APXS) is strongly affected by the presence of very light elements such as oxygen which cannot be detected directly by the APXS. C/R values are determined along with element concentrations by fitting APXS spectra of geochemical reference materials (GRMs) with the GUAPX code. A quantity K is defined as the ratio between the C/R value determined by Monte Carlo simulation based on the measured element concentrations and the fitted C/R value from the spectrum. To ensure optimally accurate K values, the choice of appropriate GRMs is explored in detail, with attention paid to Rb and Sr, whose characteristic Kα X-ray peaks overlap the Pu Lα scatter peaks. The resulting relationship between the ratio K and the overall oxygen fraction is linear. This provides a calibration from which the concentration of additional light invisible constituents (ALICs) such as water may be estimated in unknown rock and conglomerate samples. Several GRMs are used as 'unknowns' in order to evaluate the accuracy of ALIC concentrations derived in this manner.

  18. Refinement of the Compton-Rayleigh scatter ratio method for use on the Mars Science Laboratory alpha particle X-ray spectrometer

    NASA Astrophysics Data System (ADS)

    Campbell, J. L.; Perrett, G. M.; Maxwell, J. A.; Nield, E.; Gellert, R.; King, P. L.; Lee, M.; O'Meara, J. M.; Pradler, I.

    2013-05-01

    Spectra from the Mars rover alpha particle X-ray spectrometers contain the elastic and inelastic scatter peaks of the plutonium L X-rays emitted by the instrument's 244Cm source. Various spectrum fitting approaches are tested using the terrestrial twin of the APXS instrument on the Mars Science Laboratory Curiosity rover, in order to provide accurate extraction of the Lα and Lβ Compton/Rayleigh intensity ratios, which can provide information about light "invisible" constituents such as water in geological samples. A well-defined dependence of C/R ratios upon mean sample atomic number is established using a large and varied set of geochemical reference materials, and the accuracy of this calibration is examined. Detailed attention is paid to the influence of the rubidium and strontium peaks which overlap the Lα scatter peaks. Our Monte Carlo simulation code for prediction of C/R ratios from element concentrations is updated. The ratio between measured and simulated C/R ratios provides a second means of calibration.

  19. Determination of the critical premicelle concentration, first critical micelle concentration and second critical micelle concentration of surfactants by resonance Rayleigh scattering method without any probe

    NASA Astrophysics Data System (ADS)

    Shi, Yan; Luo, Hong Qun; Li, Nian Bing

    2011-05-01

    The purpose of this work is to determine the values of critical premicelle concentration (CPMC), first critical micelle concentration (FCMC) and second critical micelle concentration (SCMC) of surfactants using a common spectrofluorophotometer by recording resonance Rayleigh scattering (RRS) signal without any probe. The plot of the RRS intensities at the maximum scattering wavelength ( IRRSmax) versus surfactant concentrations ( c) was constructed to obtain the IRRSmax-c curve. From the inflexions in IRRSmax-c curve, the CPMC, FCMC and SCMC values of a surfactant can be obtained sensitively. The FCMC of some anionic, cationic and nonionic surfactants such as sodium dodecyl sulfate (SDS), sodium dodecyl benzene sulfonate (SDBS), cetyltrimethylammonium bromide (CTAB), cetylpyridinium chloride (CPC), Tween-20, and Tween-80 were determined by RRS method and the values are in good agreement with those obtained from conductivity and surface tension measurements and literature values. The CPMC and SCMC of SDS and CTAB were also determined by RRS method respectively and the values conform to literature values too. Furthermore, RRS method can also be used to determine the FCMC of an amphiphilic macromolecule-hemoglobin, whose structure resembles a surfactant. From the experimental results, it is concluded that RRS method can be applied to the simultaneous determination of the CPMC, FCMC and SCMC values in a sensitive, accurate and no probe way.

  20. Study on the interactions of antiemetic drugs and 12-tungstophosphoric acid by absorption and resonance Rayleigh scattering spectra and their analytical applications.

    PubMed

    Wang, Yaqiong; Liu, Shaopu; Liu, Zhongfang; Yang, Jidong; Hu, Xiaoli

    2013-03-15

    In 0.1 mol L(-1) HCl medium, antiemetic drugs (ATM), such as granisetron hydrochloride (GS) and tropisetron hydrochloride (TS), reacted with H(3)PW(12)O(40)·nH(2)O and formed 3:1 ion-association complex of [(ATM)(3)PW(12)O(40)], then self-aggregated into nanoparticles-[(ATM)(3)PW(12)O(40)](n) with an average size of 100 nm. The reaction resulted in the enhancement of resonance Rayleigh scattering (RRS) and the absorption spectra. The increments of scattering intensity (ΔI(RRS)) and the change of absorbance (ΔA) were both directly proportional to the concentrations of ATM in certain ranges. Accordingly, two new RRS and spectrophotometric methods were proposed for ATM detection. The detection limits (3σ) of GS and TS were 3.2 ng mL(-1) and 4.0 ng mL(-1)(RRS method), 112.5 ng mL(-1) and 100.0 ng mL(-1)(spectrophotometric method). These two methods were applied to determine GS in orally disintegrating tablets and the results were in good agreement with the official method. The ground-state geometries and electronic structures of GS and TS were optimized by the hybrid density functional theory (DFT) method and the shape of [(ATM)(3)PW(12)O(40)](n) was characterized by atomic force microscopy (AFM). Take the RRS method with higher sensitivity as an example, the reaction mechanism and the reasons for enhancement of scattering were discussed.

  1. Development of High Spectral Resolution Technique for Registration Quasielastic Light Scattering Spectra Including Rayleigh and Brillouin Scattering as a Diagnostic Tool in Materials Characterization

    DTIC Science & Technology

    2007-11-02

    develop and build an optical device, fitted to a Fabry - Perot interferometer, to perform high-resolution quasieleastic light scattering spectroscopy...scattering spectra based on the use of a scanning by gas pressure Fabry - Perot interferometer coupled to the double grating monochromator...8a. Technical Progress We have designed and built new special metallic box with two optical windows for the Fabry - Perot interferometer and fine

  2. An investigation on the interaction of DNA with hesperetin/apigenin in the presence of CTAB by resonance Rayleigh light scattering technique and its analytical application

    NASA Astrophysics Data System (ADS)

    Bi, Shuyun; Wang, Yu; Pang, Bo; Yan, Lili; Wang, Tianjiao

    2012-05-01

    Two new systems for measuring DNA at nanogram levels by a resonance Rayleigh light scattering (RLS) technique with a common spectrofluorometer were proposed. In the presence of cetyltrimethylammonium bromide (CTAB), the interaction of DNA with hesperetin and apigenin (two effective components of Chinese herbal medicine) could enhance RLS signals with the maximum peak at 363 and 433 nm respectively. The enhanced intensity of RLS was directly proportional to the concentration of DNA in the range of 0.022-4.4 μg mL-1 for DNA-CTAB-hesperetin system and 0.013-4.4 μg mL-1 for DNA-CTAB-apigenin system. The detection limit was 2.34 ng mL-1 and 2.97 ng mL-1 respectively. Synthetic samples were measured satisfactorily. The recovery of DNA-CTAB-hesperetin system was 97.3-101.9% and that of DNA-CTAB-apigenin system was 101.2-109.5%.

  3. A simple and rapid method for direct determination of Al(III) based on the enhanced resonance Rayleigh scattering of hemin-functionalized graphene-Al(III) system

    NASA Astrophysics Data System (ADS)

    Ling, Yu; Chen, Ling Xiao; Dong, Jiang Xue; Li, Nian Bing; Luo, Hong Qun

    2016-03-01

    A novel method for direct determination of Al(III) by using hemin-functionalized graphene (H-GO) has been established based on the enhancement of resonance Rayleigh scattering (RRS) intensity. The characteristics of RRS spectra, the optimum reaction conditions, and the reaction mechanism have been investigated. In this experiment, the Al(III) would exist in sol-gel Al(OH)3 species under the condition of pH 5.9 in aqueous solutions. When H-GO existed in the solution, the sol-gel Al(OH)3 would react with H-GO and result in enhancement of RRS intensity, owing to the enhanced hydrophobicity of H-GO surface. Therefore, a simple and rapid sensor for Al(III) was developed. The increased intensity of RRS is directly proportional to the concentration of Al(III) in the range of 10 nM-6 μM, along with a detection limit of 0.87 nM. Moreover, the sensor has been applied to determination of Al(III) concentration in real water and aspirin tablet samples with satisfactory results. Therefore, the proposed method is promising as an effective means for selective and sensitive determination of Al(III).

  4. A novel method for study of the aggregation of protein induced by metal ion aluminum(III) using resonance Rayleigh scattering technique

    NASA Astrophysics Data System (ADS)

    Long, Xiufen; Zhang, Caihua; Cheng, Jiongjia; Bi, Shuping

    2008-01-01

    We present a novel method for the study of the aggregation of protein induced by metal ion aluminum(III) using resonance Rayleigh scattering (RRS) technique. In neutral Tris-HCl medium, the effect of this aggregation of protein results in the enhancement of RRS intensity and the relationship between the enhancement of the RRS signal and the Al concentration is nonlinear. On this basis, we established a new method for the determination of the critical induced-aggregation concentrations ( CCIAC) of metal ion Al(III) inducing the protein aggregation. Our results show that many factors, such as, pH value, anions, salts, temperature and solvents have obvious effects. We also studied the extent of aggregation and structural changes using ultra-violet spectrometry, protein intrinsic fluorescence and circular dichroism to further understand the exact mechanisms of the aggregation characteristics of proteins induced by metal ion Al(III) at the molecular level, to help us to develop effective methods to investigate the toxicity of metal ion Al, and to provide theoretical and quantitative evidences for the development of appropriate treatments for neurodementia such as Parkinson's disease, Alzheimer's disease and dementia related to dialysis.

  5. Hydrogen bond dynamics and water structure in glucose-water solutions by depolarized Rayleigh scattering and low-frequency Raman spectroscopy

    NASA Astrophysics Data System (ADS)

    Paolantoni, Marco; Sassi, Paola; Morresi, Assunta; Santini, Sergio

    2007-07-01

    The effect of glucose on the relaxation process of water at picosecond time scales has been investigated by depolarized Rayleigh scattering (DRS) experiments. The process is assigned to the fast hydrogen bonding dynamics of the water network. In DRS spectra this contribution can be safely separated from the slower relaxation process due to the sugar. The detected relaxation time is studied at different glucose concentrations and modeled considering bulk and hydrating water contributions. As a result, it is found that in diluted conditions the hydrogen bond lifetime of proximal water molecules becomes about three times slower than that of the bulk. The effect of the sugar on the hydrogen bond water structure is investigated by analyzing the low-frequency Raman (LFR) spectrum sensitive to intermolecular modes. The addition of glucose strongly reduces the intensity of the band at 170cm-1 assigned to a collective stretching mode of water molecules arranged in cooperative tetrahedral domains. These findings indicate that proximal water molecules partially lose the tetrahedral ordering typical of the bulk leading to the formation of high density environments around the sugar. Thus the glucose imposes a new local order among water molecules localized in its hydration shell in which the hydrogen bond breaking dynamics is sensitively retarded. This work provides new experimental evidences that support recent molecular dynamics simulation and thermodynamics results.

  6. Hydrogen bond dynamics and water structure in glucose-water solutions by depolarized Rayleigh scattering and low-frequency Raman spectroscopy.

    PubMed

    Paolantoni, Marco; Sassi, Paola; Morresi, Assunta; Santini, Sergio

    2007-07-14

    The effect of glucose on the relaxation process of water at picosecond time scales has been investigated by depolarized Rayleigh scattering (DRS) experiments. The process is assigned to the fast hydrogen bonding dynamics of the water network. In DRS spectra this contribution can be safely separated from the slower relaxation process due to the sugar. The detected relaxation time is studied at different glucose concentrations and modeled considering bulk and hydrating water contributions. As a result, it is found that in diluted conditions the hydrogen bond lifetime of proximal water molecules becomes about three times slower than that of the bulk. The effect of the sugar on the hydrogen bond water structure is investigated by analyzing the low-frequency Raman (LFR) spectrum sensitive to intermolecular modes. The addition of glucose strongly reduces the intensity of the band at 170 cm(-1) assigned to a collective stretching mode of water molecules arranged in cooperative tetrahedral domains. These findings indicate that proximal water molecules partially lose the tetrahedral ordering typical of the bulk leading to the formation of high density environments around the sugar. Thus the glucose imposes a new local order among water molecules localized in its hydration shell in which the hydrogen bond breaking dynamics is sensitively retarded. This work provides new experimental evidences that support recent molecular dynamics simulation and thermodynamics results.

  7. Resonance Rayleigh Scattering Spectra of an Ion-Association Complex of Naphthol Green B-Chitosan System and Its Application in the Highly Sensitive Determination of Chitosan.

    PubMed

    Zhang, Weiai; Ma, Caijuan; Su, Zhengquan; Bai, Yan

    2016-04-18

    This work describes a highly-sensitive and accurate approach for the determination of chitosan (CTS) using Naphthol Green B (NGB) as a probe in the Resonance Rayleigh scattering (RRS) method. The interaction between CTS and NGB leads to notable enhancement of RRS, and the enhancement is proportional to the concentration of CTS over a certain range. Under optimum conditions, the calibration curve of ΔI against CTS concentration was ΔI = 1860.5c + 86.125 (c, µg/mL), R² = 0.9999, and the linear range and detection limit (DL) were 0.01-5.5 µg/mL and 8.87 ng/mL. Moreover, the effect of the molecular weight of CTS on the accurate quantification of CTS was studied. The experimental data were analyzed through linear regression analysis using SPSS20.0, and the molecular weight was found to have no statistical significance. This method has been applied to assay two CTS samples and obtained good recovery and reproducibility.

  8. Development of a non-derivatization high-performance liquid chromatography method with resonance Rayleigh scattering detection for the detection of sisomicin in rat serum.

    PubMed

    Lu, Xin; Zhang, Dan; Liu, Chengwei; Xu, Qin; Zhao, Shulin

    2009-12-01

    A resonance Rayleigh scattering (RRS) detection approach was developed to detect sisomicin (Siso) in rat serum following chromatographic separation. The detection principle is based on the enhancement of RRS intensity of ion-association complex formed from aminoglycosides and pontamine sky blue (PSB) used as molecular recognition probe. The high-performance liquid chromatography (HPLC) coupled with RRS detection scheme was implemented post-column by mixing a PSB solution with the column eluent prior to detection. The RRS signal was detected by fluorescence detector at lambda(ex)=lambda(em)=365 nm. Separation and detection conditions were optimized. Siso and etimicin (Eti) chosen as the internal standard (IS) were separated on a C(18) reversed phase column with the mobile phase consisting of a ternary mixture of 20mM sodium acetate aqueous solution-methanol (92:8, v/v) containing 0.22% TFA (v/v). The limit of detection (S/N=3) for Siso was 18 ng. A calibration curve ranged from 25 ng to 700 ng shown to be linear. The presented method was applied for the determination of Siso in rat serum and used for the pharmacokinetics study of Siso in rat.

  9. The fluorescence and resonance Rayleigh scattering spectra study on the interactions of palladium (II)-Nootropic chelate with Congo red and their analytical applications

    NASA Astrophysics Data System (ADS)

    Chen, Fang; Peng, Jingdong; Liu, Shaopu; Peng, Huanjun; Pan, Ziyu; Bu, Lingli; Xiao, Huan; Zhang, Ruiwen

    2017-04-01

    A highly sensitive detection approach of resonance Rayleigh scattering spectra (RRS) is firstly applied to analyzing nootropic drugs including piracetam (PIR) and oxiracetam (OXI). In HCl-NaAc buffer solution (pH = 3.0), the OXI chelated with palladium (II) to form the chelate cation [Pd2·OXI]2 +, and then reacted with Congo red (CGR) by virtue of electrostatic attraction and hydrophobic force to form binary complex [Pd2·OXI]. CGR2, which could result in the great enhancement of RRS. The resonance Rayleigh scattering signal was recorded at λex = λem = 375 nm. This mixture complex not only has higher RRS, but also makes contribution to significant increase of fluorescence, and the same phenomena also were discovered in PIR. The enhanced RRS intensity is in proportion to the PIR and OXI concentration in the range of 0.03-3.0 μg mL- 1, and the detection limit (DL) of RRS method for PIR and OXI is 2.3 ng mL- 1 and 9.7 ng mL- 1. In addition, the DL of fluorescence method for PIR and OXI is 8.4 μg mL- 1 and 19.5 μg mL- 1. Obviously, the RRS is the highly sensitive method, and the recoveries of the two kinds of nootropic drugs were range from 100.4% to 101.8.0% with RSD (n = 5) from 1.1% to 3.1% by RRS method. This paper not only investigated the optimum conditions for detecting nootropics with using RRS method, but also focused on the reasons for enhancing RRS intensity and the reaction mechanism, which in order to firm and contract the resultant. Finally, The RRS method has been applied to detect nootropic drugs in human urine samples with satisfactory results. Fig. S2. The effect of ionic strength: Pd (II)-CGR system (curve a); Pd (II)-OXI-CGR system (curve b); Pd (II)-PIR- CGR system (curve c). Pd (II): 2.0 × 10- 4 mol L- 1; CGR: 1.0 × 10- 5 mol L- 1; OXI: 1.5 μg mL- 1; PIR: 2 μg mL- 1; NaCl: 1 mol L- 1. Fig. S3. The effect of time: Pd (II)-OXI-CGR system (curve a); Pd (II)-PIR-CGR system (curve b). Pd (II): 2.0 × 10- 4 mol L- 1; CGR: 1.0 × 10- 5 mol L- 1

  10. Interaction of cetylpyridine bromide with nucleic acids and determination of nucleic acids at nanogram levels based on the enhancement of resonance Rayleigh light scattering.

    PubMed

    Liu, Rutao; Yang, Jinghe; Wu, Xia

    2002-07-01

    Resonance Rayleigh light scattering (RRLS) spectra of cetylpyridine bromide (CPB)-nucleic acid system and their analytical application have been first studied. The effective factors and optimum conditions of the reaction have been investigated. After CPB and nucleic acid are mixed together, a new absorption peak located at 300 nm appeared, which is due to the formation of new ion associate of CPB-nucleic acid. The new associate can result in two apparent RRLS peaks at 310-400 and 460-480 nm. The RRLS peak of the corrected spectra located at 290-350 nm, which indicate that the RRLS is originated from the absorption of CPB-nucleic acid associate. The peak at 460-480 nm disappears in the corrected RRLS spectra, which indicated that this peak is originated from the strong line emission of the Xe lamp. Under the optimum conditions, the enhanced intensity of RRLS is proportional to the concentration of nucleic acid in the range of 5.0 x 10(-9)-5.0 x 10(-5) g ml(-1) for calf thymus DNA (ctDNA), 1.0 x 10(-8)-4.0 x 10(-5) g ml(-1) for fish sperm DNA (fsDNA) and 1.0 x 10(-8)-5.0 x 10(-5) g ml(-1) for yeast RNA (yRNA). The detection limits (S/N = 3) are 4.3, 8.7 and 7.4 ng ml(-1), respectively. Synthetic samples were determined satisfactorily.

  11. Sign change of the Soret coefficient of poly(ethylene oxide) in water/ethanol mixtures observed by thermal diffusion forced Rayleigh scattering.

    PubMed

    Kita, Rio; Wiegand, Simone; Luettmer-Strathmann, Jutta

    2004-08-22

    Soret coefficients of the ternary system of poly(ethylene oxide) in mixed water/ethanol solvent were measured over a wide solvent composition range by means of thermal diffusion forced Rayleigh scattering. The Soret coefficient S(T) of the polymer was found to change sign as the water content of the solvent increases with the sign change taking place at a water mass fraction of 0.83 at a temperature of 22 degrees C. For high water concentrations, the value of S(T) of poly(ethylene oxide) is positive, i.e., the polymer migrates to the cooler regions of the fluid, as is typical for polymers in good solvents. For low water content, on the other hand, the Soret coefficient of the polymer is negative, i.e., the polymer migrates to the warmer regions of the fluid. Measurements for two different polymer concentrations showed a larger magnitude of the Soret coefficient for the smaller polymer concentration. The temperature dependence of the Soret coefficient was investigated for water-rich polymer solutions and revealed a sign change from negative to positive as the temperature is increased. Thermodiffusion experiments were also performed on the binary mixture water/ethanol. For the binary mixtures, the Soret coefficient of water was observed to change sign at a water mass fraction of 0.71. This is in agreement with experimental results from the literature. Our results show that specific interactions (hydrogen bonds) between solvent molecules and between polymer and solvent molecules play an important role in thermodiffusion for this system.

  12. On the neutral points in Rayleigh transfer

    NASA Astrophysics Data System (ADS)

    Viik, T.

    2017-03-01

    In this paper we consider the dependence of the existence and position of the neutral points on the albedo of single scattering and the optical thickness in a Rayleigh scattering plane-parallel homogeneous atmospheres. We use the Chandrasekhar method of discrete ordinates and the method of approximating the Sobolev resolvent function to solve the vector equation of transfer in l- and r-representation. On the basis of many different models of Rayleigh atmospheres we show the behaviour of the neutral points while the parallel incident flux can be both unpolarized or polarized. Our calculations show with high probability that the maximum number of neutral points in a Rayleigh atmosphere is four.

  13. Rayleigh imaging in spectral mammography

    NASA Astrophysics Data System (ADS)

    Berggren, Karl; Danielsson, Mats; Fredenberg, Erik

    2016-03-01

    Spectral imaging is the acquisition of multiple images of an object at different energy spectra. In mammography, dual-energy imaging (spectral imaging with two energy levels) has been investigated for several applications, in particular material decomposition, which allows for quantitative analysis of breast composition and quantitative contrast-enhanced imaging. Material decomposition with dual-energy imaging is based on the assumption that there are two dominant photon interaction effects that determine linear attenuation: the photoelectric effect and Compton scattering. This assumption limits the number of basis materials, i.e. the number of materials that are possible to differentiate between, to two. However, Rayleigh scattering may account for more than 10% of the linear attenuation in the mammography energy range. In this work, we show that a modified version of a scanning multi-slit spectral photon-counting mammography system is able to acquire three images at different spectra and can be used for triple-energy imaging. We further show that triple-energy imaging in combination with the efficient scatter rejection of the system enables measurement of Rayleigh scattering, which adds an additional energy dependency to the linear attenuation and enables material decomposition with three basis materials. Three available basis materials have the potential to improve virtually all applications of spectral imaging.

  14. Lord Rayleigh: John William Strutt, third Baron Rayleigh.

    PubMed

    Wells, Peter N T

    2007-03-01

    John William Strutt, first son of the second Baron Rayleigh, was born on November 12, 1842. He was a sickly boy, so his schooling was sporadic. Nevertheless, he graduated first in his year at Cambridge and subsequently was a Fellow of Trinity College until his marriage in 1871. His father died in 1873, and he succeeded to the title third Baron Rayleigh. He converted the stable block of his country house, Terling Place, into a laboratory. In 1879, he moved back to Cambridge as Professor of Experimental Physics, but he returned to Terling in 1884. He published The Theory of Sound in 1877/1878 and, in his lifetime, 466 scientific articles. He received the 1904 Nobel Prize in Physics for the discovery of argon and made numerous seminal contributions to scientific progress. In the field of acoustics, he studied scattering, the diffraction limit, surface waves, resonance phenomena, reciprocity, streaming, radiation force, cavitation, relaxation, and binaural perception. He received many honors, was President of the Royal Society, one of the founding members of the Order of Merit, and Chancellor of Cambridge University. He also was interested in psychical research. Lord Rayleigh died on June 30, 1919.

  15. Ultrasensitive Label-Free Resonance Rayleigh Scattering Aptasensor for Hg(2+) Using Hg(2+)-Triggered Exonuclease III-Assisted Target Recycling and Growth of G-Wires for Signal Amplification.

    PubMed

    Ren, Wang; Zhang, Ying; Chen, Hong Guo; Gao, Zhong Feng; Li, Nian Bing; Luo, Hong Qun

    2016-01-19

    A novel signal-on and label-free resonance Rayleigh scattering (RRS) aptasensor was constructed for detection of Hg(2+) based on Hg(2+)-triggered Exonuclease III-assisted target recycling and growth of G-quadruplex nanowires (G-wires) for signal amplification. The hairpin DNA (H-DNA) was wisely designed with thymine-rich recognition termini and a G-quadruplex sequence in the loop and employed as a signal probe for specially recognizing trace Hg(2+) by a stable T-Hg(2+)-T structure, which automatically triggered Exonuclease III (Exo-III) digestion to recycle Hg(2+) and liberate the G-quadruplex sequence. The free G-quadruplex sequences were self-assembled into guanine nanowire (G-wire) superstructure in the presence of Mg(2+) and demonstrated by gel electrophoresis. The RRS intensity was dramatically amplified by the resultant G-wires, and the maximum RRS signal at 370 nm was linear with the logarithm of Hg(2+) concentration in the range of 50.0 pM to 500.0 nM (R = 0.9957). Selectivity experiments revealed that the as-prepared RRS sensor was specific for Hg(2+), even coexisting with high concentrations of other metal ions. This optical aptasensor was successfully applied to identify Hg(2+) in laboratory tap water and river water samples. With excellent sensitivity and selectivity, the proposed RRS aptasensor was potentially suitable for not only routine detection of Hg(2+) in environmental monitoring but also various target detection just by changing the recognition sequence of the H-DNA probe.

  16. Cooperative stimulated Brillouin and Rayleigh backscattering process in optical fiber.

    PubMed

    Fotiadi, A A; Kiyan, R V

    1998-12-01

    We observed an unusually narrow spectrum of Stokes field and Gaussian statistics of Stokes power for the stimulated Brillouin scattering (SBS) process in 300-m single-mode optical fiber with high Rayleigh losses. The measured characteristics of the Stokes radiation indicate that SBS lasing took place in the fiber. The effect is explained as the result of dynamic distributed feedback that is due to double Rayleigh scattering (RS) of the Stokes field. The results of numerical simulation of the cooperative SBS-RS process in fiber are in good agreement with experimental results.

  17. Passive retrieval of Rayleigh waves in disordered elastic media.

    PubMed

    Larose, Eric; Derode, Arnaud; Clorennec, Dominique; Margerin, Ludovic; Campillo, Michel

    2005-10-01

    When averaged over sources or disorder, cross correlation of diffuse fields yields the Green's function between two passive sensors. This technique is applied to elastic ultrasonic waves in an open scattering slab mimicking seismic waves in the Earth's crust. It appears that the Rayleigh wave reconstruction depends on the scattering properties of the elastic slab. Special attention is paid to the specific role of bulk to Rayleigh wave coupling, which may result in unexpected phenomena, such as a persistent time asymmetry in the diffuse regime.

  18. Relation between the Rayleigh equation in diffraction theory and the equation based on Green's formula

    NASA Astrophysics Data System (ADS)

    Tatarskii, V. I.

    1995-06-01

    The steps necessary to produce the Rayleigh equation that is based on the Rayleigh hypothesis from the equation that is based on the Green's formula are shown. First a definition is given for the scattering amplitude that is true not only in the far zone of diffraction but also near the scattering surface. With this definition the Rayleigh equation coincides with the rigorous equation for the surface secondary sources that is based on Green's formula. The Rayleigh hypothesis is equivalent to substituting the far-zone expression of the scattering amplitude into this rigorous equation. In this case it turns out to be the equation not for the sources but directly for the scattering amplitude, which is the main advantage of this method. For comparing the Rayleigh equation with the initial rigorous equation, the Rayleigh equation is represented in terms of secondary sources. The kernel of this equation contains an integral that converges for positive and diverges for negative values of some parameter. It is shown that if we regularize this integral, defining it for the negative values of this parameter as an analytical continuation from the domain of positive values, this kernel becomes equal to the kernel of the initial rigorous equation. It follows that the formal perturbation series for the scattering amplitude obtained from the Rayleigh equation and from Green's equation always coincide. This means that convergence of the perturbation series is a sufficient condition

  19. Strutt, John William [Lord Rayleigh] (1842-1919)

    NASA Astrophysics Data System (ADS)

    Murdin, P.

    2000-11-01

    Born in Langford Grove (near Maldon), Essex, England, Nobel prizewinner (1904) for the discovery of argon. He worked in many areas of physics, including electromagnetism and sound; the Rayleigh theory of the scattering of light was the first correct explanation of why the sky is blue....

  20. Microwave scattering from laser spark in air

    SciTech Connect

    Sawyer, Jordan; Zhang Zhili; Shneider, Mikhail N.

    2012-09-15

    In this paper, microwave Mie scattering from a laser-induced plasma in atmospheric air is computed. It shows that the scattered microwave transitions from coherent Rayleigh scattering to Mie scattering based on the relative transparency of the laser-induced plasma at the microwave frequency. The microwave penetration in the plasma alters from total transparency to partial shielding due to the sharp increase of the electron number density within the avalanche ionization phase. The transition from Rayleigh scattering to Mie scattering is verified by both the temporal evolution of the scattered microwave and the homogeneity of polar scattering plots.

  1. Characterization of Surface Cracks Using Rayleigh Waves

    SciTech Connect

    Masserey, B.; Mazza, E.

    2005-04-09

    The characterization of surface cracks in steel plates using surface acoustic waves is investigated. In the experiments Rayleigh wave is generated by a standard wedge technique and the surface displacement is measured pointwise by means of a heterodyne laser interferometer. The presence of a crack in the acoustic field leads to an amplitude increase due to the scattering of the surface wave at the defect. The time-of-flight method is extended to crack depth smaller than the wavelength by correlating the time delay of the transmitted wave with the defect depth. The method is shown to provide good results for defect depths down to 0.2 mm.

  2. The Rayleigh Papers

    NASA Astrophysics Data System (ADS)

    Miller, Thomas; Bederson, Benjamin

    2005-04-01

    The Third Lord Rayleigh (1842-1919), aka John William Strutt, was among the most stellar physicists of the Nineteenth Century, in both theory and experiment. He spent most of his mature years in his own laboratory, self-funded, on his family estate. One of the consequences was the fact that all of his papers remained at the estate upon his death. After his son's (Robert John Strutt, 1875-1947) death both their scientific papers ended up on the auction block. (Robert John was himself an atmospheric physicist.) Part of the Strutt collection went to the Burndy Library of the Dibner Institute at MIT, but most landed in the library at the US Air Force Cambridge Research Laboratory (now the Air Force Research Laboratory at Hansom AFB), purchased from the auctioneer out of library funds, for 9,000. The individual most responsible for preserving these papers was John N. Howard, the laboratory Chief Scientist, who was a founding editor of the journal Applied Optics. Recently the authors examined first hand the Rayleigh papers. Included in these are a complete set of his handwritten scientific notes, taken over the period 1862-1919, from the time he was a student at Trinity College, Cambridge until just months before his death. We will show a number of interesting examples from these notes, including his first identification of argon, as well as some other fascinating items from the collection.

  3. Microscopic Rayleigh Droplet Beams

    NASA Astrophysics Data System (ADS)

    Doak, R. B.

    2005-11-01

    A periodically triggered Rayleigh Droplet Beam (RDB) delivers a perfectly linear and periodic stream of identical, monoenergetic droplets that are phase-locked to the trigger signal. The droplet diameter and spacing are easily adjusted of choice of nozzle diameter and trigger frequency. Any liquid of low viscosity may be emloyed as the beam fluid. Although the field of nanofluidics is expanding rapidly, little effort has yet been devoted to ``external flows'' such as RDB's. At ASU we have generated RDB's of water and methanol down to 2 microns in droplet diameter. Nozzle clogging is the sole impediment to smaller droplets. Microscopic Rayleigh droplet beams offer tremendous potential for fundamental physical measurements, fluid dynamics research, and nanofabrication. This talk will describe the apparatus and techniques used at ASU to generate RDB's (surprisingly simple and inexpensive), discuss the triboelectric phenomena that play a role (surprisingly significant), present some initial experimental fluid dynamics measurements, and briefly survey RDB applications. Our particular interest in RDB's is as microscopic transport systems to deliver hydrated, undenatured proteins into vacuum for structure determination via serial diffraction of x-rays or electrons. This may offer the first general method for structure determination of non-crystallizable proteins.

  4. Rayleigh Laser Guide Star Systems: Application to the University of Illinois Seeing Improvement System

    NASA Astrophysics Data System (ADS)

    Thompson, Laird A.; Teare, Scott W.

    2002-09-01

    Laser guide stars created by Rayleigh scattering provide a reasonable means to monitor atmospheric wavefront distortions for real-time correction by adaptive optics systems. Because of the λ-4 wavelength dependence of Rayleigh scattering, short-wavelength lasers are a logical first choice for astronomical laser guide star systems, and in this paper we describe the results from a sustained experimental effort to integrate into an adaptive optics system a 351 nm Rayleigh laser guide star created at an altitude of 20 km (above mean sea level) at the Mount Wilson 2.5 m telescope. In addition to providing obvious scientific benefits, the 351 nm laser guide star projected by the University of Illinois Seeing Improvement System is ``stealth qualified'' in terms of the Federal Aviation Administration and airplane avoidance. Because of the excellent return signal at the wavefront sensor, there is no doubt that future applications will be found for short-wavelength Rayleigh-scattered laser guide stars.

  5. Rayleigh radiance computations for satellite remote sensing: accounting for the effect of sensor spectral response function.

    PubMed

    Wang, Menghua

    2016-05-30

    To understand and assess the effect of the sensor spectral response function (SRF) on the accuracy of the top of the atmosphere (TOA) Rayleigh-scattering radiance computation, new TOA Rayleigh radiance lookup tables (LUTs) over global oceans and inland waters have been generated. The new Rayleigh LUTs include spectral coverage of 335-2555 nm, all possible solar-sensor geometries, and surface wind speeds of 0-30 m/s. Using the new Rayleigh LUTs, the sensor SRF effect on the accuracy of the TOA Rayleigh radiance computation has been evaluated for spectral bands of the Visible Infrared Imaging Radiometer Suite (VIIRS) on the Suomi National Polar-orbiting Partnership (SNPP) satellite and the Joint Polar Satellite System (JPSS)-1, showing some important uncertainties for VIIRS-SNPP particularly for large solar- and/or sensor-zenith angles as well as for large Rayleigh optical thicknesses (i.e., short wavelengths) and bands with broad spectral bandwidths. To accurately account for the sensor SRF effect, a new correction algorithm has been developed for VIIRS spectral bands, which improves the TOA Rayleigh radiance accuracy to ~0.01% even for the large solar-zenith angles of 70°-80°, compared with the error of ~0.7% without applying the correction for the VIIRS-SNPP 410 nm band. The same methodology that accounts for the sensor SRF effect on the Rayleigh radiance computation can be used for other satellite sensors. In addition, with the new Rayleigh LUTs, the effect of surface atmospheric pressure variation on the TOA Rayleigh radiance computation can be calculated precisely, and no specific atmospheric pressure correction algorithm is needed. There are some other important applications and advantages to using the new Rayleigh LUTs for satellite remote sensing, including an efficient and accurate TOA Rayleigh radiance computation for hyperspectral satellite remote sensing, detector-based TOA Rayleigh radiance computation, Rayleigh radiance calculations for high altitude

  6. Based on coherent detection of Rayleigh - Brillouin temperature measurement

    NASA Astrophysics Data System (ADS)

    Zheng, Yeliang; Hu, Yihua; Huang, Baokun

    2016-11-01

    The traditional laser temperature measurement usually adopt the direct detection method, while the direct detection method is easily influenced by aerosol scattering and background stray light. In this paper, the DSC710 balanced detector was first applied to the measurement of complete gas Rayleigh - Brillouin scattering spectrum (RBS). By utilizing the difference of RBS spectrum broadening under different temperature to get the temperature information. In this article, a simple theoretical derivation and error analysis has been made. The results show that using this method can effectively inhibit the interference of background stray light and has high precision.

  7. Energy conservation - A test for scattering approximations

    NASA Technical Reports Server (NTRS)

    Acquista, C.; Holland, A. C.

    1980-01-01

    The roles of the extinction theorem and energy conservation in obtaining the scattering and absorption cross sections for several light scattering approximations are explored. It is shown that the Rayleigh, Rayleigh-Gans, anomalous diffraction, geometrical optics, and Shifrin approximations all lead to reasonable values of the cross sections, while the modified Mie approximation does not. Further examination of the modified Mie approximation for the ensembles of nonspherical particles reveals additional problems with that method.

  8. Multi-Component, Multi-Point Interferometric Rayleigh/Mie Doppler Velocimeter

    NASA Technical Reports Server (NTRS)

    Danehy, Paul M.; Lee, Joseph W.; Bivolaru, Daniel

    2012-01-01

    An interferometric Rayleigh scattering system was developed to enable the measurement of multiple, orthogonal velocity components at several points within very-high-speed or high-temperature flows. The velocity of a gaseous flow can be optically measured by sending laser light into the gas flow, and then measuring the scattered light signal that is returned from matter within the flow. Scattering can arise from either gas molecules within the flow itself, known as Rayleigh scattering, or from particles within the flow, known as Mie scattering. Measuring Mie scattering is the basis of all commercial laser Doppler and particle imaging velocimetry systems, but particle seeding is problematic when measuring high-speed and high-temperature flows. The velocimeter is designed to measure the Doppler shift from only Rayleigh scattering, and does not require, but can also measure, particles within the flow. The system combines a direct-view, large-optic interferometric setup that calculates the Doppler shift from fringe patterns collected with a digital camera, and a subsystem to capture and re-circulate scattered light to maximize signal density. By measuring two orthogonal components of the velocity at multiple positions in the flow volume, the accuracy and usefulness of the flow measurement increase significantly over single or nonorthogonal component approaches.

  9. Rayleigh-Taylor Shock Waves

    SciTech Connect

    Olson, B J; Cook, A W

    2007-08-30

    Beginning from a state of hydrostatic equilibrium, in which a heavy gas rests atop a light gas in a constant gravitational field, Rayleigh-Taylor instability at the interface will launch a shock wave into the upper fluid. The rising bubbles of lighter fluid act like pistons, compressing the heavier fluid ahead of the fronts and generating shocklets. These shocklets coalesce in multidimensional fashion into a strong normal shock, which increases in strength as it propagates upwards. Large-eddy simulations demonstrate that the shock Mach number increases faster in three dimensions than it does in two dimensions. The generation of shocks via Rayleigh-Taylor instability could have profound implications for astrophysical flows.

  10. Rotating Rayleigh-Taylor turbulence

    NASA Astrophysics Data System (ADS)

    Boffetta, G.; Mazzino, A.; Musacchio, S.

    2016-09-01

    The turbulent Rayleigh-Taylor system in a rotating reference frame is investigated by direct numerical simulations within the Oberbeck-Boussinesq approximation. On the basis of theoretical arguments, supported by our simulations, we show that the Rossby number decreases in time, and therefore the Coriolis force becomes more important as the system evolves and produces many effects on Rayleigh-Taylor turbulence. We find that rotation reduces the intensity of turbulent velocity fluctuations and therefore the growth rate of the temperature mixing layer. Moreover, in the presence of rotation the conversion of potential energy into turbulent kinetic energy is found to be less effective, and the efficiency of the heat transfer is reduced. Finally, during the evolution of the mixing layer we observe the development of a cyclone-anticyclone asymmetry.

  11. Time-sequenced and spectrally filtered Rayleigh imaging of shock wave and boundary layer structure for inlet characterization

    NASA Technical Reports Server (NTRS)

    Forkey, Joseph; Cogne, Sandrine; Smits, Alexander; Bogdonoff, Seymour; Lempert, Walter R.; Miles, Richard B.

    1993-01-01

    Multiple pulsed Rayleigh imaging and filtered Rayleigh scattering are used to generate images of a complex boundary layer structure, shock wave/boundary layer interactions, and crossing shock waves. Time-sequenced Rayleigh images taken with a visible, double-pulsed laser system show the evolution of boundary layer structure of the internal flow in a generic cross-shock inlet. The images taken in the inlet give insight into 3D effects caused by the inlet geometry and may be used for modeling the complex flows.

  12. Simulating the Rayleigh-Taylor instability with the Ising model

    SciTech Connect

    Ball, Justin R.; Elliott, James B.

    2011-08-26

    The Ising model, implemented with the Metropolis algorithm and Kawasaki dynamics, makes a system with its own physics, distinct from the real world. These physics are sophisticated enough to model behavior similar to the Rayleigh-Taylor instability and by better understanding these physics, we can learn how to modify the system to better re ect reality. For example, we could add a vx and a vy to each spin and modify the exchange rules to incorporate them, possibly using two body scattering laws to construct a more realistic system.

  13. Asymptotic Rayleigh instantaneous unit hydrograph

    USGS Publications Warehouse

    Troutman, B.M.; Karlinger, M.R.

    1988-01-01

    The instantaneous unit hydrograph for a channel network under general linear routing and conditioned on the network magnitude, N, tends asymptotically, as N grows large, to a Rayleigh probability density function. This behavior is identical to that of the width function of the network, and is proven under the assumption that the network link configuration is topologically random and the link hydraulic and geometric properties are independent and identically distributed random variables. The asymptotic distribution depends only on a scale factor, {Mathematical expression}, where ?? is a mean link wave travel time. ?? 1988 Springer-Verlag.

  14. Rotating Rayleigh-Taylor instability

    NASA Astrophysics Data System (ADS)

    Scase, M. M.; Baldwin, K. A.; Hill, R. J. A.

    2017-02-01

    The effect of rotation upon the classical Rayleigh-Taylor instability is investigated. We consider a two-layer system with an axis of rotation that is perpendicular to the interface between the layers. In general, we find that a wave mode's growth rate may be reduced by rotation. We further show that in some cases, unstable axisymmetric wave modes may be stabilized by rotating the system above a critical rotation rate associated with the mode's wavelength, the Atwood number, and the flow's aspect ratio.

  15. Light scattering from nonspherical airborne particles: Experimental and theoretical comparisons

    NASA Astrophysics Data System (ADS)

    Hirst, Edwin; Kaye, Paul H.; Guppy, John R.

    1994-10-01

    Spatial intensity distribution of laser light scattered by airborne hazardous particles such as asbestos fiber is studied to classify particles shape and size. Theoretical treatment is based on Rayleigh-Gans formalism. Theoretical and experimental data are in good agreement.

  16. Nonideal Rayleigh-Taylor mixing

    SciTech Connect

    Sharp, David Howland; Lin, Hyun K; Iwerks, Justin G; Gliman, James G

    2009-01-01

    Rayleigh-Taylor mixing is a classical hydrodynamic Instability, which occurs when a light fluid pushes against a heavy fluid. The two main sources of nonideal behavior in Rayleigh-Taylor (RT) mixing are regularizations (physical and numerical) which produce deviations from a pure Euler equation, scale Invariant formulation, and non Ideal (i.e. experimental) initial conditions. The Kolmogorov theory of turbulence predicts stirring at all length scales for the Euler fluid equations without regularization. We Interpret mathematical theories of existence and non-uniqueness in this context, and we provide numerical evidence for dependence of the RT mixing rate on nonideal regularizations, in other words indeterminacy when modeled by Euler equations. Operationally, indeterminacy shows up as non unique solutions for RT mixing, parametrized by Schmidt and Prandtl numbers, In the large Reynolds number (Euler equation) limit. Verification and validation evidence is presented for the large eddy simulation algorithm used here. Mesh convergence depends on breaking the nonuniqueness with explicit use of the laminar Schmidt and PrandtJ numbers and their turbulent counterparts, defined in terms of subgrid scale models. The dependence of the mixing rate on the Schmidt and Prandtl numbers and other physical parameters will be illustrated. We demonstrate numerically the influence of initial conditions on the mixing rate. Both the dominant short wavelength Initial conditions and long wavelength perturbations are observed to playa role. By examination of two classes of experiments, we observe the absence of a single universal explanation, with long and short wavelength initial conditions, and the various physical and numerical regularizations contributing In different proportions In these two different contexts.

  17. Experimental Investigation of Scattering from Randomly Rough Plastic Cylinders

    DTIC Science & Technology

    1992-09-01

    fluid, here following the form from Morse and Ingard [20] and Skudrzyk [21]. First, the adiabatic equation of state relating the pressure, p, and...wavelength, we get the standard relation between the particle velocity and the pressure u = -VP. (2.6) Rayleigh [19] and Morse and Ingard [20] derive the...the internal and scattered fields, Rayleigh [191 and Morse and Ingard [20] solve for the scattered field from an infinitely long circular cylinder by

  18. Matrix operator theory of radiative transfer. I - Rayleigh scattering.

    NASA Technical Reports Server (NTRS)

    Plass, G. N.; Kattawar, G. W.; Catchings, F. E.

    1973-01-01

    An entirely rigorous method for the solution of the equations for radiative transfer based on the matrix operator theory is reviewed. The advantages of the present method are: (1) all orders of the reflection and transmission matrices are calculated at once; (2) layers of any thickness may be combined, so that a realistic model of the atmosphere can be developed from any arbitrary number of layers, each with different properties and thicknesses; (3) calculations can readily be made for large optical depths and with highly anisotropic phase functions; (4) results are obtained for any desired value of the surface albedo including the value unity and for a large number of polar and azimuthal angles; (5) all fundamental equations can be interpreted immediately in terms of the physical interactions appropriate to the problem; and (6) both upward and downward radiance can be calculated at interior points from relatively simple expressions.

  19. A study of compressible mixing layers using filtered Rayleigh scattering

    NASA Technical Reports Server (NTRS)

    Elliott, Gregory S.; Samimy, MO; Arnette, Stephen A.

    1992-01-01

    High Reynolds number compressible planar free shear layers were studied using a planar laser visualization technique. Two convective Mach numbers, M(c) = 0.51 and 0.86, were studied in the developing and fully developed regions. The structures in the M(c) = 0.51 case were characterized by 2D core and roller regions, similar to subsonic shear layers. Also for the M(c) = 0.51 case, plan views in the developing region showed the existence of streamwise streaks, possibly indicating the presence of organized streamwise vorticity. The M(c) = 0.86 flow was much less organized than the lower convective Mach number case and highly three dimensional.

  20. Filtered Rayleigh Scattering Measurements in a Buoyant Flowfield

    DTIC Science & Technology

    2007-03-01

    is presented in Figure 32 and Figure 33. The sampli rate is 6.5 Hz with an exposure time of 50 ms. The downstream location is 0.8 inches (x/d = 3.1...FRS signal can be collected using a 10 m manufacturer suggests a sampli A 50 ms exposure time is chosen in this res of processing the data and is a

  1. Depolarization Ratio of Rayleigh Scattered Radiation by Molecules

    DTIC Science & Technology

    2007-01-12

    the constraint imposed by the conservation of 2 angular momentum to be 1/4, the high temperature value of X C(1 la;M,q - M) (3) the vector coupling...the Clebsch-Gordan (vector coupling) coefficient; - ) ’,( ) ’ I(aji,jf) X 12(a), (1) C 2(jiajf ;0,0) ensures the conservation of angular momen- dfl2 C...Meath15 we obtain Po,= 2 .6posed by the conservation of angular momentum are absent. X 10-3, 1/4 times the measured value of (0.96±_0.14) Table I gives six

  2. Leaky Rayleigh wave ultrasonic backscattering enhancements: Experimental tests of theory for tilted solid cylinders and cubes

    NASA Astrophysics Data System (ADS)

    Gipson, Karen

    Backscattering enhancements due to acoustic wave coupling into leaky Rayleigh waves on solid elastic cubes and cylinders submerged in water are investigated. A quantitative ray description of the launching and propagation of the leaky Rayleigh waves is verified to be useful. Leaky Rayleigh waves are launched on the surface of an elastic object if the acoustic wavevector's projection along the surface matches the wavevector associated with leaky Rayleigh wave propagation. Once launched, leaky Rayleigh waves on the surface of an elastic object will be partially reflected at the object's truncations, and under certain conditions the reflection process may result in a reversal of the leaky wavevector on the surface so that the leaky radiation is oriented in the backscattering direction. Furthermore, the radiated wavefront can have a vanishing Gaussian curvature which produces a far-field caustic. The leaky wave pressure on the surface of the scatterer is approximated by convolving the incident pressure with an appropriate function describing the response of the surface to a localized pressure input, and the method of images is used to approximate the reflection processes. The resulting reflected pressure field on or near the target's surface is then propagated to the far field using the Rayleigh-Sommerfeld diffraction integral. Tone burst experiments confirm that this approach provides reasonable predictions for a variety of cases including the retroreflection of leaky waves around a comer on the face of a cube, the retroreflection of meridional leaky waves along the length of a cylinder, and the retroreflection of leaky waves launched diagonally across the flat face of a cylinder. The frequency dependence of these mechanisms for backscattering from a cylinder was also investigated using a pressure source capable of producing an impulsive pressure, and the observed time returns for end-reflected helical waves agree with theoretical predictions. For the high frequencies

  3. Measurements of density, pressure and temperature in the middle atmosphere with Rayleigh lidar

    NASA Astrophysics Data System (ADS)

    Deng, Pan; Zhang, Tianshu; Chen, Wei; Liu, Jianguo

    2016-10-01

    Ground-based observations of the middle atmospheric density, pressure and temperature profiles can be obtained by lidar. A single-wavelength Rayleigh lidar system based at Hefei (31°N,117°E) has been used to measure the atmospheric density, pressure and temperature in the middle atmosphere in night in the altitude range from about 25 to 40 km. The structure of Rayleigh lidar system, principles of middle atmospheric density, pressure and temperature measurement which is based on the Rayleigh scattering theory and method to retrieve atmospheric density, pressure and temperature profiles were described respectively. This instrument combined a 500mW Nd:YAG laser transmitter with a 0.4 m receiver mirror to observe returns from altitudes between 25km and 40km.The lidar observed atmosphere density, pressure and temperature profiles are validated through comparison with the measure data provided by sounding balloon. According to the data from actual measurement, the inversion of the vertical distribution of middle atmosphere density, pressure and temperature are in good agreement with the result of sounding balloon. Generally, in the altitude range 25 to 40 km, the density ratio profile of Rayleigh lidar to the sounding balloon density fluctuates between 0.98 and 1.10, the pressure ratio profile of Rayleigh lidar to the sounding balloon is between 0.99 and 1.06 and the deviation of the temperature is less than 6 k.

  4. High Prandtl number effect on Rayleigh-Bénard convection heat transfer at high Rayleigh number

    NASA Astrophysics Data System (ADS)

    Ma, Li; Li, Jing; Ji, Shui; Chang, Huajian

    2017-02-01

    This paper represents results of the Rayleigh-Bénard convection heat transfer in silicon oil confined by two horizontal plates, heated from below, and cooled from above. The Prandtl numbers considered as 100-10,000 corresponding to three types of silicon oil. The experiments covered a range of Rayleigh numbers from 2.14·109 to 2.27·1013. The data points that the Nusselt number dependents on the Rayleigh number, which is asymptotic to a 0.248 power. Furthermore, the experiment results can fit the data in low Rayleigh number well.

  5. Chemical oscillator as a generalized Rayleigh oscillator

    NASA Astrophysics Data System (ADS)

    Ghosh, Shyamolina; Ray, Deb Shankar

    2013-10-01

    We derive the conditions under which a set of arbitrary two dimensional autonomous kinetic equations can be reduced to the form of a generalized Rayleigh oscillator which admits of limit cycle solution. This is based on a linear transformation of field variables which can be found by inspection of the kinetic equations. We illustrate the scheme with the help of several chemical and bio-chemical oscillator models to show how they can be cast as a generalized Rayleigh oscillator.

  6. Ultraviolet Rayleigh-Mie lidar for daytime-temperature profiling of the troposphere

    NASA Astrophysics Data System (ADS)

    Hua, Dengxin; Uchida, Masaru; Kobayashi, Takao

    2005-03-01

    A UV Rayleigh-Mie scattering lidar has been developed for daytime measurement of temperature and aerosol optical properties in the troposphere. The transmitter is a narrowband, injection-seeded, pulsed, third-harmonic Nd:YAG laser at an eye-safe wavelength of 355 nm. Two Fabry-Perot etalons (FPEs) with a dual-pass optical layout filter the molecular Rayleigh scattering components spectrally for retrieval of the temperature and provide a high rejection rate for aerosol Mie scattering in excess of 43 dB. The Mie signal is filtered with a third FPE filter for direct profiling of aerosol optical properties. The Mie scattering component in the Rayleigh signals, which will have influence on temperature measurements, is corrected by using a measure of aerosol scattering because of the relative insufficiency of Mie rejection of Rayleigh filters in the presence of dense aerosols or clouds, and the Mie rejection capability of system is thus improved. A narrowband interference filter is incorporated with the FPEs to block solar radiation. Also, the small field of view (0.1 mrad) of the receiver and the UV wavelength used enhance the ability of the lidar to suppress the solar background signal in daytime measurement. The system is relatively compact, with a power-aperture product of 0.18 W m^-2, and has a high sensitivity to temperature change (0.62%/K). Lidar measurements taken under different weather conditions (winter and summer) are demonstrated. Good agreement between the lidar and the radiosonde measurements was obtained in terms of lapse rates and inversions. Statistical temperature errors of less than 1 K up to a height of 2 km are obtainable, with an averaging time of ~12 min for daytime measurements.

  7. Ultraviolet Rayleigh-Mie lidar for daytime-temperature profiling of the troposphere.

    PubMed

    Hua, Dengxin; Uchida, Masaru; Kobayashi, Takao

    2005-03-01

    A UV Rayleigh-Mie scattering lidar has been developed for daytime measurement of temperature and aerosol optical properties in the troposphere. The transmitter is a narrowband, injection-seeded, pulsed, third-harmonic Nd:YAG laser at an eye-safe wavelength of 355 nm. Two Fabry-Perot etalons (FPEs) with a dual-pass optical layout filter the molecular Rayleigh scattering components spectrally for retrieval of the temperature and provide a high rejection rate for aerosol Mie scattering in excess of 43 dB. The Mie signal is filtered with a third FPE filter for direct profiling of aerosol optical properties. The Mie scattering component in the Rayleigh signals, which will have influence on temperature measurements, is corrected by using a measure of aerosol scattering because of the relative insufficiency of Mie rejection of Rayleigh filters in the presence of dense aerosols or clouds, and the Mie rejection capability of system is thus improved. A narrowband interference filter is incorporated with the FPEs to block solar radiation. Also, the small field of view (0.1 mrad) of the receiver and the UV wavelength used enhance the ability of the lidar to suppress the solar background signal in daytime measurement. The system is relatively compact, with a power-aperture product of 0.18 W m(-2), and has a high sensitivity to temperature change (0.62%/K). Lidar measurements taken under different weather conditions (winter and summer) are demonstrated. Good agreement between the lidar and the radiosonde measurements was obtained in terms of lapse rates and inversions. Statistical temperature errors of less than 1 K up to a height of 2 km are obtainable, with an averaging time of approximately 12 min for daytime measurements.

  8. Rayleigh--Taylor spike evaporation

    SciTech Connect

    Schappert, G. T.; Batha, S. H.; Klare, K. A.; Hollowell, D. E.; Mason, R. J.

    2001-09-01

    Laser-based experiments have shown that Rayleigh--Taylor (RT) growth in thin, perturbed copper foils leads to a phase dominated by narrow spikes between thin bubbles. These experiments were well modeled and diagnosed until this '' spike'' phase, but not into this spike phase. Experiments were designed, modeled, and performed on the OMEGA laser [T. R. Boehly, D. L. Brown, R. S. Craxton , Opt. Commun. 133, 495 (1997)] to study the late-time spike phase. To simulate the conditions and evolution of late time RT, a copper target was fabricated consisting of a series of thin ridges (spikes in cross section) 150 {mu}m apart on a thin flat copper backing. The target was placed on the side of a scale-1.2 hohlraum with the ridges pointing into the hohlraum, which was heated to 190 eV. Side-on radiography imaged the evolution of the ridges and flat copper backing into the typical RT bubble and spike structure including the '' mushroom-like feet'' on the tips of the spikes. RAGE computer models [R. M. Baltrusaitis, M. L. Gittings, R. P. Weaver, R. F. Benjamin, and J. M. Budzinski, Phys. Fluids 8, 2471 (1996)] show the formation of the '' mushrooms,'' as well as how the backing material converges to lengthen the spike. The computer predictions of evolving spike and bubble lengths match measurements fairly well for the thicker backing targets but not for the thinner backings.

  9. Rayleigh-Taylor mixing in supernova experiments

    SciTech Connect

    Swisher, N. C.; Abarzhi, S. I.; Kuranz, C. C.; Arnett, D.; Hurricane, O.; Remington, B. A.; Robey, H. F.

    2015-10-15

    We report a scrupulous analysis of data in supernova experiments that are conducted at high power laser facilities in order to study core-collapse supernova SN1987A. Parameters of the experimental system are properly scaled to investigate the interaction of a blast-wave with helium-hydrogen interface, and the induced Rayleigh-Taylor instability and Rayleigh-Taylor mixing of the denser and lighter fluids with time-dependent acceleration. We analyze all available experimental images of the Rayleigh-Taylor flow in supernova experiments and measure delicate features of the interfacial dynamics. A new scaling is identified for calibration of experimental data to enable their accurate analysis and comparisons. By properly accounting for the imprint of the experimental conditions, the data set size and statistics are substantially increased. New theoretical solutions are reported to describe asymptotic dynamics of Rayleigh-Taylor flow with time-dependent acceleration by applying theoretical analysis that considers symmetries and momentum transport. Good qualitative and quantitative agreement is achieved of the experimental data with the theory and simulations. Our study indicates that in supernova experiments Rayleigh-Taylor flow is in the mixing regime, the interface amplitude contributes substantially to the characteristic length scale for energy dissipation; Rayleigh-Taylor mixing keeps order.

  10. Quantitative Scattering of Melanin Solutions

    NASA Astrophysics Data System (ADS)

    Riesz, J.; Gilmore, J.; Meredith, P.

    2006-06-01

    The optical scattering coefficient of a dilute, well solubilised eumelanin solution has been accurately measured as a function of incident wavelength, and found to contribute less than 6% of the total optical attenuation between 210 and 325nm. At longer wavelengths (325nm to 800nm) the scattering was less than the minimum sensitivity of our instrument. This indicates that UV and visible optical density spectra can be interpreted as true absorption with a high degree of confidence. The scattering coefficient vs wavelength was found to be consistent with Rayleigh Theory for a particle radius of 38+-1nm.

  11. Rayleigh Quotient Iteration in 3D, Deterministic Neutron Transport

    SciTech Connect

    Slaybaugh, R; Evans, Thomas M; Davidson, Gregory G; Wilson, P.

    2012-01-01

    Today's "grand challenge" neutron transport problems require 3-D meshes with billions of cells, hundreds of energy groups, and accurate quadratures and scattering expansions. Leadership-class computers provide platforms on which high-fidelity fluxes can be calculated. However, appropriate methods are needed that can use these machines effectively. Such methods must be able to use hundreds of thousands of cores and have good convergence properties. Rayleigh quotient iteration (RQI) is an eigenvalue solver that has been added to the Sn code Denovo to address convergence. Rayleigh quotient iteration is an optimal shifted inverse iteration method that should converge in fewer iterations than the more common power method and other shifted inverse iteration methods for many problems of interest. Denovo's RQI uses a new multigroup Krylov solver for the fixed source solutions inside every iteration that allows parallelization in energy in addition to space and angle. This Krylov solver has been shown to scale successfully to 200,000 cores: for example one test problem scaled from 69,120 cores to 190,080 cores with 98% efficiency. This paper shows that RQI works for some small problems. However, the Krylov method upon which it relies does not always converge because RQI creates ill-conditioned systems. This result leads to the conclusion that preconditioning is needed to allow this method to be applicable to a wider variety of problems.

  12. Possibility of modification of the Rayleigh line in a nonequilibrium fluid with a constant shear velocity gradient

    NASA Astrophysics Data System (ADS)

    Sahoo, Debendranath; Sood, A. K.

    1984-11-01

    We show that the recent prediction of the García-Colín and Velasco

    [Phys. Rev. A 26 2187 (1982)]
    regarding the modification of the Rayleigh line, in the scattering of light from a fluid kept under a constant shear veloity gradient, is incorrect. A correct application of fluctuating hydrodynamics is shown to predict no such change.

  13. Supershear Rayleigh Waves at a Soft Interface

    NASA Astrophysics Data System (ADS)

    Le Goff, Anne; Cobelli, Pablo; Lagubeau, Guillaume

    2013-06-01

    We report on the experimental observation of waves at a liquid foam surface propagating faster than the bulk shear waves. The existence of such waves has long been debated, but the recent observation of supershear events in a geophysical context has inspired us to search for their existence in a model viscoelastic system. An optimized fast profilometry technique allows us to observe on a liquid foam surface the waves triggered by the impact of a projectile. At high impact velocity, we show that the expected subshear Rayleigh waves are accompanied by faster surface waves that can be identified as supershear Rayleigh waves.

  14. Doppler optical mixing spectroscopy in multiparticle scattering fluids

    SciTech Connect

    Dubnishchev, Yu N

    2011-03-31

    We discuss the basic scheme of laser Doppler optical mixing spectroscopy for the analysis of media with multiparticle scattering. It is shown that the Rayleigh scheme, in contrast to the heterodyne and differential schemes, is insensitive to the effects of multiparticle scattering. (laser applications and other aspects of quantum electronics)

  15. Experimental confirmation of neoclassical Compton scattering theory

    SciTech Connect

    Aristov, V. V.; Yakunin, S. N.; Despotuli, A. A.

    2013-12-15

    Incoherent X-ray scattering spectra of diamond and silicon crystals recorded on the BESSY-2 electron storage ring have been analyzed. All spectral features are described well in terms of the neoclassical scattering theory without consideration for the hypotheses accepted in quantum electrodynamics. It is noted that the accepted tabular data on the intensity ratio between the Compton and Rayleigh spectral components may significantly differ from the experimental values. It is concluded that the development of the general theory (considering coherent scattering, incoherent scattering, and Bragg diffraction) must be continued.

  16. Laser Rayleigh and Raman Diagnostics for Small Hydrogen/oxygen Rockets

    NASA Technical Reports Server (NTRS)

    Degroot, Wilhelmus A.; Zupanc, Frank J.

    1993-01-01

    Localized velocity, temperature, and species concentration measurements in rocket flow fields are needed to evaluate predictive computational fluid dynamics (CFD) codes and identify causes of poor rocket performance. Velocity, temperature, and total number density information have been successfully extracted from spectrally resolved Rayleigh scattering in the plume of small hydrogen/oxygen rockets. Light from a narrow band laser is scattered from the moving molecules with a Doppler shifted frequency. Two components of the velocity can be extracted by observing the scattered light from two directions. Thermal broadening of the scattered light provides a measure of the temperature, while the integrated scattering intensity is proportional to the number density. Spontaneous Raman scattering has been used to measure temperature and species concentration in similar plumes. Light from a dye laser is scattered by molecules in the rocket plume. Raman spectra scattered from major species are resolved by observing the inelastically scattered light with linear array mounted to a spectrometer. Temperature and oxygen concentrations have been extracted by fitting a model function to the measured Raman spectrum. Results of measurements on small rockets mounted inside a high altitude chamber using both diagnostic techniques are reported.

  17. Laser Rayleigh and Raman diagnostics for small hydrogen/oxygen rockets

    NASA Astrophysics Data System (ADS)

    Degroot, Wilhelmus A.; Zupanc, Frank J.

    1993-01-01

    Localized velocity, temperature, and species concentration measurements in rocket flow fields are needed to evaluate predictive computational fluid dynamics (CFD) codes and identify causes of poor rocket performance. Velocity, temperature, and total number density information have been successfully extracted from spectrally resolved Rayleigh scattering in the plume of small hydrogen/oxygen rockets. Light from a narrow band laser is scattered from the moving molecules with a Doppler shifted frequency. Two components of the velocity can be extracted by observing the scattered light from two directions. Thermal broadening of the scattered light provides a measure of the temperature, while the integrated scattering intensity is proportional to the number density. Spontaneous Raman scattering has been used to measure temperature and species concentration in similar plumes. Light from a dye laser is scattered by molecules in the rocket plume. Raman spectra scattered from major species are resolved by observing the inelastically scattered light with linear array mounted to a spectrometer. Temperature and oxygen concentrations have been extracted by fitting a model function to the measured Raman spectrum. Results of measurements on small rockets mounted inside a high altitude chamber using both diagnostic techniques are reported.

  18. Laser Rayleigh and Raman diagnostics for small hydrogen/oxygen rockets

    NASA Astrophysics Data System (ADS)

    de Groot, Wim A.; Zupanc, Frank J.

    1993-05-01

    Localized velocity, temperature, and species concentration measurements in rocket flow fields are needed to evaluate predictive computational fluid dynamics (CFD) codes and identify causes of poor rocket performance. Velocity, temperature, and total number density information have been successfully extracted from spectrally resolved Rayleigh scattering in the plume of small hydrogen/oxygen rockets. Light from a narrow band laser is scattered from the moving molecules with a Doppler shifted frequency. Two components of the velocity can be extracted by observing the scattered light from two directions. Thermal broadening of the scattered light provides a measure of the temperature, while the integrated scattering intensity is proportional to the number density. Spontaneous Raman scattering has been used to measure temperature and species concentration in similar plumes. Light from a dye laser is scattered by molecules in the rocket plume. Raman spectra scattered from major species are resolved by observing the inelastically scattered light with a linear array mounted to a spectrometer. Temperature and oxygen concentrations have been extracted by fitting a model function to the measured Raman spectrum. Results of measurements on small rockets mounted inside a high altitude chamber using both diagnostic techniques are reported.

  19. Light Scattering from Exoplanet Oceans and Atmospheres

    NASA Astrophysics Data System (ADS)

    Zugger, Michael; Kasting, J. F.; Williams, D. M.; Kane, T. J.; Philbrick, C. R.

    2011-01-01

    Orbital variation in reflected starlight from exoplanets could eventually be used to detect surface oceans. Exoplanets with rough surfaces, or dominated by atmospheric Rayleigh scattering, should reach peak brightness in full phase, orbital longitude = 180deg, whereas ocean planets with transparent atmospheres should reach peak brightness in crescent phase near OL = 30deg. Application of Fresnel theory to a planet with no atmosphere covered by a calm ocean predicts a peak polarization fraction of 1 at OL = 74deg; however, our model shows that clouds, wind-driven waves, aerosols, absorption, and Rayleigh scattering in the atmosphere and within the water column, dilute the polarization fraction and shift the peak to other OLs. Observing at longer wavelengths reduces the obfuscation of the water polarization signature by Rayleigh scattering but does not mitigate the other effects. Planets with thick Rayleigh scattering atmospheres reach peak polarization near OL = 90deg, but clouds and Lambertian surface scattering dilute and shift this peak to smaller OL. A shifted Rayleigh peak might be mistaken for a water signature unless data from multiple wavelength bands are available. Our calculations suggest that polarization alone may not positively identify the presence of an ocean under an Earth-like atmosphere; however polarization adds another dimension which can be used, in combination with unpolarized orbital light curves and contrast ratios, to detect extrasolar oceans, atmospheric water aerosols, and water clouds. Additionally, the presence and direction of the polarization vector could be used to determine planet association with the star, and constrain orbit inclination. This research was funded by the NASA Astrobiology Institute, the University of Washington Virtual Planetary Laboratory, and the Penn State Astrobiology Institute. Authors M. Zugger, J. Kasting, and D. Williams are members of the Penn State Center for Exoplanets and Habitable Worlds.

  20. Low scattering loss fiber with segmented-core and depressed inner cladding structure

    NASA Astrophysics Data System (ADS)

    Pournoury, Marzieh; Moon, Dae Seung; Nazari, Tavakol; Kassani, Sahar Hosseinzadeh; Do, Mun-Hyun; Lee, Yeong Seop; Oh, Kyunghwan

    2014-04-01

    In this paper, using the FEM method new low-loss fiber is proposed to minimize Rayleigh scattering with a segmented-core and depressed inner-cladding. The optical loss of the designed fiber is calculated based on Rayleigh scattering losses. Rayleigh scattering loss (RSL) has been estimated by Rayleigh scattering coefficient (RSC) and power distribution in the fiber. We have shown loss of less than 0.3 dB/km at 1310 nm, 0.18 dB/km at 1550 nm for step-index fibers which consist of conventional glass compositions such as SiO2, GeO2-SiO2, F-SiO2 while satisfying all of ITU-G.652.D attributes.

  1. Use of Rayleigh imaging and ray tracing to correct for beam-steering effects in turbulent flames.

    PubMed

    Kaiser, Sebastian A; Frank, Jonathan H; Long, Marshall B

    2005-11-01

    Laser Rayleigh imaging has been applied in a number of flow and flame studies to measure concentration or temperature distributions. Rayleigh cross sections are dependent on the index of refraction of the scattering medium. The same index of refraction changes that provide contrast in Rayleigh images can also deflect the illuminating laser sheet. By applying a ray-tracing algorithm to the detected image, it is possible to correct for some of these beam-steering effects and thereby improve the accuracy of the measured field. Additionally, the quantification of the degree of beam steering through the flow provides information on the degradation of spatial resolution in the measurement. Application of the technique in a well-studied laboratory flame is presented, along with analysis of the effects of image noise and spatial resolution on the effectiveness of the algorithm.

  2. Experimental and theoretical study of Rayleigh-Lamb waves in a plate containing a surface-breaking crack

    NASA Technical Reports Server (NTRS)

    Paffenholz, Joseph; Fox, Jon W.; Gu, Xiaobai; Jewett, Greg S.; Datta, Subhendu K.

    1990-01-01

    Scattering of Rayleigh-Lamb waves by a normal surface-breaking crack in a plate has been studied both theoretically and experimentally. The two-dimensionality of the far field, generated by a ball impact source, is exploited to characterize the source function using a direct integration technique. The scattering of waves generated by this impact source by the crack is subsequently solved by employing a Green's function integral expression for the scattered field coupled with a finite element representation of the near field. It is shown that theoretical results of plate response, both in frequency and time, are similar to those obtained experimentally. Additionally, implication for practical applications are discussed.

  3. Rayleigh-Taylor Mix experiment on Pegasus

    SciTech Connect

    Sheppard, M.G.; Atchison, W.L.; Anderson, W.E.

    1997-09-01

    The Rayleigh-Taylor Mix project will attempt to diagnose and understand the growth of a mixing layer at the interface between an imploding metal liner and a polystyrene foam core in a series of pulsed power experiments on the Pegasus capacitor bank. Understanding the effects of material strength will be an important part of the study. During the initial phase of the implosion, the linear/foam interface is Rayleigh-Taylor (RT) stable; however, as the foam is compressed, it decelerates the liner, causing it to bound and to go RT unstable. This paper reports 1D and 2D MHD simulations of the first experiment in the series and preliminary results.

  4. Rayleigh instability at small length scales

    NASA Astrophysics Data System (ADS)

    Gopan, Nandu; Sathian, Sarith P.

    2014-09-01

    The Rayleigh instability (also called the Plateau-Rayleigh instability) of a nanosized liquid propane thread is investigated using molecular dynamics (MD). The validity of classical predictions at small length scales is verified by comparing the temporal evolution of liquid thread simulated by MD against classical predictions. Previous works have shown that thermal fluctuations become dominant at small length scales. The role and influence of the stochastic nature of thermal fluctuations in determining the instability at small length scale is also investigated. Thermal fluctuations are seen to dominate and accelerate the breakup process only during the last stages of breakup. The simulations also reveal that the breakup profile of nanoscale threads undergo modification due to reorganization of molecules by the evaporation-condensation process.

  5. Magnetically Induced Rotating Rayleigh-Taylor Instability.

    PubMed

    Scase, Matthew M; Baldwin, Kyle A; Hill, Richard J A

    2017-03-03

    Classical techniques for investigating the Rayleigh-Taylor instability include using compressed gasses(1), rocketry(2) or linear electric motors(3) to reverse the effective direction of gravity, and accelerate the lighter fluid toward the denser fluid. Other authors(e.g.)(4)(,)(5)(,)(6) have separated a gravitationally unstable stratification with a barrier that is removed to initiate the flow. However, the parabolic initial interface in the case of a rotating stratification imposes significant technical difficulties experimentally. We wish to be able to spin-up the stratification into solid-body rotation and only then initiate the flow in order to investigate the effects of rotation upon the Rayleigh-Taylor instability. The approach we have adopted here is to use the magnetic field of a superconducting magnet to manipulate the effective weight of the two liquids to initiate the flow. We create a gravitationally stable two-layer stratification using standard flotation techniques. The upper layer is less dense than the lower layer and so the system is Rayleigh-Taylor stable. This stratification is then spun-up until both layers are in solid-body rotation and a parabolic interface is observed. These experiments use fluids with low magnetic susceptibility, |χ| ~ 10(-6) - 10(-5), compared to a ferrofluids. The dominant effect of the magnetic field applies a body-force to each layer changing the effective weight. The upper layer is weakly paramagnetic while the lower layer is weakly diamagnetic. When the magnetic field is applied, the lower layer is repelled from the magnet while the upper layer is attracted towards the magnet. A Rayleigh-Taylor instability is achieved with application of a high gradient magnetic field. We further observed that increasing the dynamic viscosity of the fluid in each layer, increases the length-scale of the instability.

  6. High-frequency Rayleigh-wave method

    USGS Publications Warehouse

    Xia, J.; Miller, R.D.; Xu, Y.; Luo, Y.; Chen, C.; Liu, J.; Ivanov, J.; Zeng, C.

    2009-01-01

    High-frequency (???2 Hz) Rayleigh-wave data acquired with a multichannel recording system have been utilized to determine shear (S)-wave velocities in near-surface geophysics since the early 1980s. This overview article discusses the main research results of high-frequency surface-wave techniques achieved by research groups at the Kansas Geological Survey and China University of Geosciences in the last 15 years. The multichannel analysis of surface wave (MASW) method is a non-invasive acoustic approach to estimate near-surface S-wave velocity. The differences between MASW results and direct borehole measurements are approximately 15% or less and random. Studies show that simultaneous inversion with higher modes and the fundamental mode can increase model resolution and an investigation depth. The other important seismic property, quality factor (Q), can also be estimated with the MASW method by inverting attenuation coefficients of Rayleigh waves. An inverted model (S-wave velocity or Q) obtained using a damped least-squares method can be assessed by an optimal damping vector in a vicinity of the inverted model determined by an objective function, which is the trace of a weighted sum of model-resolution and model-covariance matrices. Current developments include modeling high-frequency Rayleigh-waves in near-surface media, which builds a foundation for shallow seismic or Rayleigh-wave inversion in the time-offset domain; imaging dispersive energy with high resolution in the frequency-velocity domain and possibly with data in an arbitrary acquisition geometry, which opens a door for 3D surface-wave techniques; and successfully separating surface-wave modes, which provides a valuable tool to perform S-wave velocity profiling with high-horizontal resolution. ?? China University of Geosciences (Wuhan) and Springer-Verlag GmbH 2009.

  7. Helium Atom Scattering as a Probe of Surface Phonons.

    NASA Astrophysics Data System (ADS)

    Yerkes, Steven Charles

    A low energy (15-63 meV) helium beam is scattered from two different crystal surfaces; mechanically cleaved and polished LiF(100), and epitaxially grown Ag(111). Conservation equations for total particle energy and parallel momentum are presented as the basis for understanding the scattering experiment. These equations along with the system response function are used to numerically model the inelastic scattering data. The scattering of helium from LiF(100) at a surface temperature of approximately 140(DEGREES)K is reported along the <010> and <110> directions. Coherent elastic scattering intensities are used for surface characterization. Over 80% of the coherent inelastic scattering can be accounted for by the interaction with single Rayleigh phonons, and is consistent with a calculated rigid-ion Rayleigh phonon dispersion relation of LiF(100). These conclusions are supported by over 85 separate inelastic experiments performed at two incident beam energies (62.5 meV and 20.5 meV) and at several incident angles (50(DEGREES), 60(DEGREES), 65(DEGREES), 70(DEGREES)). The scattering from single Rayleigh phonons is reported as a function of crystal surface temperature, scattering angle, phonon frequency, and azimuthal angle. The inelastic scattering data is compared with the calculated intensities of an analytic inelastic scattering theory. The surface temperature dependent inelastic scattering intensity of the data are qualitatively predicted by the theory, however, the theory is inadequate in predicting the experimental intensity as a function of scattering angle, phonon frequency, and azimuthal angle. Incoherent elastic scattering (due to surface defects) is also reported as a function of scattered angle. No existing theory can account for the observed behavior of this scattering. Preliminary coherent inelastic scattering data are reported for. 23 meV helium from Ag(111) directed 12.5(DEGREES) from the <112>. Single(' ). Rayleigh phonons account for less than 60% of

  8. Modeling stray light from rough surfaces and subsurface scatter

    NASA Astrophysics Data System (ADS)

    Harvey, James E.; Goshy, John J.; Pfisterer, Richard N.

    2014-09-01

    Over the years we have developed an adequate theory and understanding of surface scatter from smooth optical surfaces (Rayleigh-Rice), moderately rough surfaces with paraxial incident and scattered angles (Beckmann- Kirchhoff) and even for moderately rough surfaces with arbitrary incident and scattered angles where a linear systems formulation requiring a two-parameter family of surface transfer functions is required to characterize the surface scatter process (generalized Harvey-Shack). However, there is always some new material or surface manufacturing process that provides non-intuitive scatter behavior. The linear systems formulation of surface scatter is potentially useful even for these situations. In this paper we will present empirical models of several classes of rough surfaces or materials (subsurface scatter) that allow us to accurately model the scattering behavior at any incident angle from limited measured scatter data. In particular, scattered radiance appears to continue being the natural quantity that exhibits simple, elegant behavior only in direction cosine space.

  9. Gaining improved chemical composition by exploitation of Compton-to-Rayleigh intensity ratio in XRF analysis.

    PubMed

    Hodoroaba, Vasile-Dan; Rackwitz, Vanessa

    2014-07-15

    The high specificity of the coherent (Rayleigh), as well as incoherent (Compton) X-ray scattering to the mean atomic number of a specimen to be analyzed by X-ray fluorescence (XRF), is exploited to gain more information on the chemical composition. Concretely, the evaluation of the Compton-to-Rayleigh intensity ratio from XRF spectra and its relation to the average atomic number of reference materials via a calibration curve can reveal valuable information on the elemental composition complementary to that obtained from the reference-free XRF analysis. Particularly for matrices of lower mean atomic numbers, the sensitivity of the approach is so high that it can be easily distinguished between specimens of mean atomic numbers differing from each other by 0.1. Hence, the content of light elements which are "invisible" for XRF, particularly hydrogen, or of heavier impurities/additives in light materials can be calculated "by difference" from the scattering calibration curve. The excellent agreement between such an experimental, empirical calibration curve and a synthetically generated one, on the basis of a reliable physical model for the X-ray scattering, is also demonstrated. Thus, the feasibility of the approach for given experimental conditions and particular analytical questions can be tested prior to experiments with reference materials. For the present work a microfocus X-ray source attached on an SEM/EDX (scanning electron microscopy/energy dispersive X-ray spectroscopy) system was used so that the Compton-to-Rayleigh intensity ratio could be acquired with EDX spectral data for improved analysis of the elemental composition.

  10. Definition of the Rayleigh number for geodynamo simulation

    NASA Astrophysics Data System (ADS)

    Kono, Masaru; Roberts, Paul H.

    2001-12-01

    A single nondimensional parameter, the Rayleigh number, suffices to characterize the onset of convection in a fluid layer of constant thickness. Geodynamo simulations concern much more complicated situations in which the fluid motions occur in a rapidly rotating sphere or spherical shell. The governing equations can be scaled in more than one way, and this leads to several alternative definitions of the Rayleigh number. Immediate comparisons between results that use different scalings and different definitions of the Rayleigh number become impossible, and confusions can arise. In this paper, ways of avoiding ambiguity are described, and a preferred definition of the Rayleigh number is proposed that is particularly well-suited for geodynamo simulations.

  11. Mitigation of Rayleigh crosstalk using noise suppression technique in 10-Gb/s REAM-SOA.

    PubMed

    Jeong, Jong Sool; Kim, Hyun-Soo; Choi, Byung-Seok; Kim, Dong Churl; Kim, Ki-Soo; Park, Mi-Ran; Kwon, O-Kyun

    2012-11-19

    We demonstrate a mitigation of Rayleigh back-scattering (RBS) impact in 10-Gb/s reflective electroabsorption modulator monolithically integrated with semiconductor optical amplifier (REAM-SOA). The technique is based on the intensity-noise suppression of the centralized incoherent seed-light, which enables smooth evolution of deployed DWDM applications. We exhibit the power penalty of less than 1 dB at the large RBS crosstalk value of about 8 dB when the optical power of seed-light is lowered about -10 dBm.

  12. Rayleigh beacon for measuring the surface profile of a radio telescope.

    PubMed

    Padin, S

    2014-12-01

    Millimeter-wavelength Rayleigh scattering from water droplets in a cloud is proposed as a means of generating a bright beacon for measuring the surface profile of a radio telescope. A λ=3  mm transmitter, with an output power of a few watts, illuminating a stratiform cloud, can generate a beacon with the same flux as Mars in 10 GHz bandwidth, but the beacon has a narrow line width, so it is extremely bright. The key advantage of the beacon is that it can be used at any time, and positioned anywhere in the sky, as long as there are clouds.

  13. Tunable multiwavelength narrow linewidth Brillouin erbium fiber laser based on Rayleigh backscattering

    NASA Astrophysics Data System (ADS)

    Wang, Xiaorui; Yang, Yanfu; Liu, Meng; Yao, Yong

    2016-06-01

    A Rayleigh backscattering (RBS) assisted Brillouin erbium fiber laser scheme with multiwavelength narrow linewidth output is proposed and investigated experimentally. The stimulated Brillouin scattering and RBS take place at two conventional single-mode fibers (SMFs), respectively. RBS is used as a mechanism to compress the linewidth of each Stokes component, and it has been realized and maximized in conventional SMF by optimizing injection power of Stokes light through adjusting variable optical attenuator (VOA). By adjusting VOA attenuation, the laser can obtain three wavelengths output with 3 dB linewidth less than 2 KHz for each wavelength, or six wavelengths output with 3 dB linewidth less than 5 KHz.

  14. Imaging Rayleigh wave attenuation with USArray

    NASA Astrophysics Data System (ADS)

    Bao, Xueyang; Dalton, Colleen A.; Jin, Ge; Gaherty, James B.; Shen, Yang

    2016-07-01

    The EarthScope USArray provides an opportunity to obtain detailed images of the continental upper mantle at an unprecedented scale. The majority of mantle models derived from USArray data to date contain spatial variations in seismic-wave speed; however, in many cases these data sets do not by themselves allow a non-unique interpretation. Joint interpretation of seismic attenuation and velocity models can improve upon the interpretations based only on velocity and provide important constraints on the temperature, composition, melt content, and volatile content of the mantle. The surface wave amplitudes that constrain upper-mantle attenuation are sensitive to factors in addition to attenuation, including the earthquake source excitation, focusing and defocusing by elastic structure, and local site amplification. Because of the difficulty of isolating attenuation from these other factors, little is known about the attenuation structure of the North American upper mantle. In this study, Rayleigh wave traveltime and amplitude in the period range 25-100 s are measured using an interstation cross-correlation technique, which takes advantage of waveform similarity at nearby stations. Several estimates of Rayleigh wave attenuation and site amplification are generated at each period, using different approaches to separate the effects of attenuation and local site amplification on amplitude. It is assumed that focusing and defocusing effects can be described by the Laplacian of the traveltime field. All approaches identify the same large-scale patterns in attenuation, including areas where the attenuation values are likely contaminated by unmodelled focusing and defocusing effects. Regionally averaged attenuation maps are constructed after removal of the contaminated attenuation values, and the variations in intrinsic shear attenuation that are suggested by these Rayleigh wave attenuation maps are explored.

  15. Investigation of the Rayleigh-Taylor and Richtmyer-Meshkov instabilities

    SciTech Connect

    Riccardo Bonazza; Mark Anderson; Leslie Smith

    2004-01-14

    Some of the major difficulties encountered in the effort to achieve nuclear fusion by means of inertial confinement arise from the unstable behavior of the interface between the shell material and the nuclear fuel which develops upon implosion of the shell by direct or indirect laser drive. The fluid flows that develop (termed the Rayleigh-Taylor (RT) and the Richtmyer-Meshkov (RM) instabilities) cause the gassified shell material to mix with the nuclear fuel, causing a reduction in energy yield or no ignition altogether. The present research program addresses the Rayleigh-Taylor and the Richtmyer-Meshkov instabilities with extensive laboratory and computational experiments. In the past year, three new activities have been initiated: a new shock tube experiment, involving the impulsive acceleration of a test gas-filled soap bubble, diagnosed with planar Mie scattering or planar induced fluorescence; a Rayleigh-Taylor experiment based on the use of a magnetorheological (MR) fluid to fix the initial shape of the interface between the MR fluid and water; and a series of computer calculations using the Raptor code (made available by Lawrence Livermore National Laboratory) to design and simulate the shock tube experiments.

  16. Vibrational energy flow models for the Rayleigh-Love and Rayleigh-Bishop rods

    NASA Astrophysics Data System (ADS)

    Han, Ju-Bum; Hong, Suk-Yoon; Song, Jee-Hun; Kwon, Hyun-Wung

    2014-01-01

    Energy Flow Analysis (EFA) has been developed to predict the vibrational energy density of the system structures in the medium-to-high frequency range. The elementary longitudinal wave theory is often used to describe the longitudinal vibration of a slender rod. However, for relatively large diameter rods or high frequency ranges, the elementary longitudinal wave theory is inaccurate because the lateral motions are not taken into account. In this paper, vibrational energy flow models are developed to analyze the longitudinally vibrating Rayleigh-Love rod considering the effect of lateral inertia, and the Rayleigh-Bishop rod considering the effect not only of the lateral inertia but also of the shear stiffness. The derived energy governing equations are second-order differential equations which predict the time and space averaged energy density and active intensity distributions in a rod. To verify the accuracy of the developed energy flow models, various numerical analyses are performed for a rod and coupled rods. Also, the EFA results for the Rayleigh-Love and Rayleigh-Bishop rods are compared with the analytical solutions for these models, the traditional energy flow solutions, and the analytical solutions for the classical rod.

  17. Predictability of Rayleigh-Taylor instability

    SciTech Connect

    Viecelli, J.A.

    1986-03-27

    Numerical experiments modeling the Rayleigh Taylor instability are carried out using a two-dimensional incompressible Eulerian hydrodynamic code VFTS. The method of integrating the Navier-Stokes equations including the viscous terms is similar to that described in Kim and Moin, except that Lagrange particles have been added and provision for body forces is given. The Eulerian method is 2nd order accurate in both space and time, and the Poisson equation for the effective pressure field is solved exactly at each time step using a cyclic reduction method. 3 refs., 3 figs.

  18. Stratospheric temperature measurement with scanning Fabry-Perot interferometer for wind retrieval from mobile Rayleigh Doppler lidar.

    PubMed

    Xia, Haiyun; Dou, Xiankang; Shangguan, Mingjia; Zhao, Ruocan; Sun, Dongsong; Wang, Chong; Qiu, Jiawei; Shu, Zhifeng; Xue, Xianghui; Han, Yuli; Han, Yan

    2014-09-08

    Temperature detection remains challenging in the low stratosphere, where the Rayleigh integration lidar is perturbed by aerosol contamination and ozone absorption while the rotational Raman lidar is suffered from its low scattering cross section. To correct the impacts of temperature on the Rayleigh Doppler lidar, a high spectral resolution lidar (HSRL) based on cavity scanning Fabry-Perot Interferometer (FPI) is developed. By considering the effect of the laser spectral width, Doppler broadening of the molecular backscatter, divergence of the light beam and mirror defects of the FPI, a well-behaved transmission function is proved to show the principle of HSRL in detail. Analysis of the statistical error of the HSRL is carried out in the data processing. A temperature lidar using both HSRL and Rayleigh integration techniques is incorporated into the Rayleigh Doppler wind lidar. Simultaneous wind and temperature detection is carried out based on the combined system at Delhi (37.371°N, 97.374°E; 2850 m above the sea level) in Qinghai province, China. Lower Stratosphere temperature has been measured using HSRL between 18 and 50 km with temporal resolution of 2000 seconds. The statistical error of the derived temperatures is between 0.2 and 9.2 K. The temperature profile retrieved from the HSRL and wind profile from the Rayleigh Doppler lidar show good agreement with the radiosonde data. Specifically, the max temperature deviation between the HSRL and radiosonde is 4.7 K from 18 km to 36 km, and it is 2.7 K between the HSRL and Rayleigh integration lidar from 27 km to 34 km.

  19. Quantum theory of Thomson scattering

    NASA Astrophysics Data System (ADS)

    Crowley, B. J. B.; Gregori, G.

    2014-12-01

    The general theory of the scattering of electromagnetic radiation in atomic plasmas and metals, in the non-relativistic regime, in which account is taken of the Kramers-Heisenberg polarization terms in the Hamiltonian, is described from a quantum mechanical viewpoint. As well as deriving the general formula for the double differential Thomson scattering cross section in an isotropic finite temperature multi-component system, this work also considers closely related phenomena such as absorption, refraction, Raman scattering, resonant (Rayleigh) scattering and Bragg scattering, and derives many essential relationships between these quantities. In particular, the work introduces the concept of scattering strength and the strength-density field which replaces the normal particle density field in the standard treatment of scattering by a collection of similar particles and it is the decomposition of the strength-density correlation function into more familiar-looking components that leads to the final result. Comparisons are made with previous work, in particular that of Chihara [1].

  20. Turbulent convection at very high Rayleigh numbers

    PubMed

    Niemela; Skrbek; Sreenivasan; Donnelly

    2000-04-20

    Turbulent convection occurs when the Rayleigh number (Ra)--which quantifies the relative magnitude of thermal driving to dissipative forces in the fluid motion--becomes sufficiently high. Although many theoretical and experimental studies of turbulent convection exist, the basic properties of heat transport remain unclear. One important question concerns the existence of an asymptotic regime that is supposed to occur at very high Ra. Theory predicts that in such a state the Nusselt number (Nu), representing the global heat transport, should scale as Nu proportional to Ra(beta) with beta = 1/2. Here we investigate thermal transport over eleven orders of magnitude of the Rayleigh number (10(6) < or = Ra < or = 10(7)), using cryogenic helium gas as the working fluid. Our data, over the entire range of Ra, can be described to the lowest order by a single power-law with scaling exponent beta close to 0.31. In particular, we find no evidence for a transition to the Ra(1/2) regime. We also study the variation of internal temperature fluctuations with Ra, and probe velocity statistics indirectly.

  1. Superstructures in Rayleigh-Benard convection

    NASA Astrophysics Data System (ADS)

    Stevens, Richard; Verzicco, Roberto; Lohse, Detlef

    2016-11-01

    We study the heat transfer and the flow structures in Rayleigh-Bénard convection as function of the Rayleigh number Ra and the aspect ratio. We consider three-dimensional direct numerical simulations (DNS) in a laterally periodic geometry with aspect ratios up to Γ =Lx /Lz =Ly /Lz = 64 at Ra =108 , where Lx and Ly indicate the horizontal domain sizes and Lz the height. We find that the heat transport convergences relatively quickly with increasing aspect ratio. In contrast, we find that the large scale flow structures change significantly with increasing aspect ratio due to the formation of superstructures. For example, at Ra =108 we find the formation of basically only one large scale circulation roll in boxes with an aspect ratio up to 8. For larger boxes we find the formation of multiple of these extremely large convection rolls. We illustrate this by movies of horizontal cross-section of the bulk and the boundary layer and analyze them by using spectra in the boundary layer and the bulk. In addition, we study the effect of the large scale flow structures on the mean and higher order temperature and velocity statistics in the boundary layer and the bulk by comparing the simulation results obtained in different aspect ratio boxes. Foundation for fundamental Research on Matter (FOM), Netherlands Center for Multiscale Catalytic Energy Conversion (MCEC), SURFsara, Gauss Large Scale project.

  2. Universality of energy spectrum in turbulent Rayleigh-Benard convection

    NASA Astrophysics Data System (ADS)

    Bai, Kunlun; Hoeller, Judith; Brown, Eric

    2016-11-01

    We present study of energy spectrum in turbulent Rayleigh-Benard convection, in both cylindrical and cubic containers, tilting and non-tilting conditions, and with Rayleigh number ranging from 0 . 5 ×109 to 1 ×1010 . For these different conditions of geometry, tilt, and Rayleigh number, the temperature spectra measured on the system side walls are significantly different from each other. Even for the same condition, the spectrum varies depending on whether the sensors locate in the path of large-scale circulations. However, quite interestingly, once the signals of large-scale circulations are subtracted from the raw temperature, all spectra display a universal shape, regardless of system geometry, tilt, Rayleigh number, and location of sensors. It suggests that one could model the large-scale circulations and small-scale fluctuations separately in turbulent Rayleigh-Benard convection.

  3. Experimental study on stimulated scattering of ZnO nanospheres dispersed in water

    NASA Astrophysics Data System (ADS)

    Shi, Jiulin; Wu, Haopeng; Yan, Feng; Yang, Junjie; He, Xingdao

    2016-01-01

    The backward stimulated scattering (BSS) from ZnO nanospheres dispersed in water has been investigated experimentally by employing a Nd:YAG pulse laser with 532 nm wavelength and 8 ns pulse width as the pump laser source. The present results show that the BSS effect is uniquely and unequivocally different compared to other known stimulated scattering, such as stimulated Rayleigh scattering, stimulated Brillouin scattering, and stimulated Raman scattering, and it displays the characteristics of no frequency shift and threshold dependence on initial spontaneous Mie scattering seed source. These can be understood by means of the Mie scattering theory and a laser-induced stationary Bragg grating model.

  4. Analytical optical scattering in clouds

    NASA Technical Reports Server (NTRS)

    Phanord, Dieudonne D.

    1989-01-01

    An analytical optical model for scattering of light due to lightning by clouds of different geometry is being developed. The self-consistent approach and the equivalent medium concept of Twersky was used to treat the case corresponding to outside illumination. Thus, the resulting multiple scattering problem is transformed with the knowledge of the bulk parameters, into scattering by a single obstacle in isolation. Based on the size parameter of a typical water droplet as compared to the incident wave length, the problem for the single scatterer equivalent to the distribution of cloud particles can be solved either by Mie or Rayleigh scattering theory. The super computing code of Wiscombe can be used immediately to produce results that can be compared to the Monte Carlo computer simulation for outside incidence. A fairly reasonable inverse approach using the solution of the outside illumination case was proposed to model analytically the situation for point sources located inside the thick optical cloud. Its mathematical details are still being investigated. When finished, it will provide scientists an enhanced capability to study more realistic clouds. For testing purposes, the direct approach to the inside illumination of clouds by lightning is under consideration. Presently, an analytical solution for the cubic cloud will soon be obtained. For cylindrical or spherical clouds, preliminary results are needed for scattering by bounded obstacles above or below a penetrable surface interface.

  5. Experiments on the rarefaction wave driven Rayleigh-Taylor instability initiated with a random initial perturbation

    NASA Astrophysics Data System (ADS)

    Morgan, Robert; Jacobs, Jeffrey

    2014-11-01

    Experiments are presented in which a diffuse interface between two gases is accelerated to become Rayleigh-Taylor unstable. The initially flat interface is generated by the opposing flow of two test gases at matched volumetric flow rates exiting through small holes in the test section. A random, three-dimensional interface perturbation is forced using a loudspeaker. The interface is then accelerated by an expansion wave which is generated by the rupturing of a diaphragm separating the heavy gas from a vacuum tank evacuated to ~0.01 atm. The expansion wave generates a large (of order 1000 g), non-constant acceleration acting on the interface causing the Rayleigh-Taylor instability to develop. Planar Mie scattering is employed to visualize the flow using a planar laser sheet generated at the top of the apparatus, which illuminates smoke particles seeded in the heavy gas. The scattered light is then recorded using a CMOS camera operating at 12 kHz. The mixing layer width is obtained from an ensemble of experiments and the turbulent growth parameter α is extracted and compared with previous experiments and simulations.

  6. Dayglow emissions of the O2 Herzberg bands and the Rayleigh backscattered spectrum of the earth

    NASA Astrophysics Data System (ADS)

    Frederick, J. E.; Abrams, R. B.

    1982-06-01

    It is pointed out that numerous fluorescent emissions from the Herzberg bands of molecular oxygen lie in the spectral region 242-300 nm. This coincides with the wavelength range used by orbiting spectrometers that observe the Rayleigh backscattered spectrum of the earth for the purpose of monitoring the vertical distribution of stratospheric ozone. Model calculations suggest that Herzberg band emissions in the dayglow could provide significant contamination of the ozone measurements if the quenching rate of O2(A3Sigma) is sufficiently small. It is noted that this is especially true near 255 nm, where the most intense fluorescent emissions relative to the Rayleigh scattered signal are located and where past satellite measurements have shown a persistent excess radiance above that expected for a pure ozone absorbing and molecular scattering atmosphere. Very small quenching rates, however, are adequate to reduce the dayglow emission to negligible levels. Noting that available laboratory data have not definitely established the quenching on the rate of O2(A3Sigma) as a function of vibration level, it is emphasized that such information is required before the Herzberg band contributions can be evaluated with confidence.

  7. Dayglow emissions of the O2 Herzberg bands and the Rayleigh backscattered spectrum of the earth

    NASA Technical Reports Server (NTRS)

    Frederick, J. E.; Abrams, R. B.

    1982-01-01

    It is pointed out that numerous fluorescent emissions from the Herzberg bands of molecular oxygen lie in the spectral region 242-300 nm. This coincides with the wavelength range used by orbiting spectrometers that observe the Rayleigh backscattered spectrum of the earth for the purpose of monitoring the vertical distribution of stratospheric ozone. Model calculations suggest that Herzberg band emissions in the dayglow could provide significant contamination of the ozone measurements if the quenching rate of O2(A3Sigma) is sufficiently small. It is noted that this is especially true near 255 nm, where the most intense fluorescent emissions relative to the Rayleigh scattered signal are located and where past satellite measurements have shown a persistent excess radiance above that expected for a pure ozone absorbing and molecular scattering atmosphere. Very small quenching rates, however, are adequate to reduce the dayglow emission to negligible levels. Noting that available laboratory data have not definitely established the quenching on the rate of O2(A3Sigma) as a function of vibration level, it is emphasized that such information is required before the Herzberg band contributions can be evaluated with confidence.

  8. Rayleigh-Taylor instability in elastic solids

    NASA Astrophysics Data System (ADS)

    Piriz, A. R.; Cela, J. J. López; Cortázar, O. D.; Tahir, N. A.; Hoffmann, D. H. H.

    2005-11-01

    We present an analytical model for the Rayleigh-Taylor instability that allows for an approximate but still very accurate and appealing description of the instability physics in the linear regime. The model is based on the second law of Newton and it has been developed with the aim of dealing with the instability of accelerated elastic solids. It yields the asymptotic instability growth rate but also describes the initial transient phase determined by the initial conditions. We have applied the model to solid/solid and solid/fluid interfaces with arbitrary Atwood numbers. The results are in excellent agreement with previous models that yield exact solutions but which are of more limited validity. Our model allows for including more complex physics. In particular, the present approach is expected to lead to a more general theory of the instability that would allow for describing the transition to the plastic regime.

  9. Rayleigh-type parametric chemical oscillation

    SciTech Connect

    Ghosh, Shyamolina; Ray, Deb Shankar

    2015-09-28

    We consider a nonlinear chemical dynamical system of two phase space variables in a stable steady state. When the system is driven by a time-dependent sinusoidal forcing of a suitable scaling parameter at a frequency twice the output frequency and the strength of perturbation exceeds a threshold, the system undergoes sustained Rayleigh-type periodic oscillation, wellknown for parametric oscillation in pipe organs and distinct from the usual forced quasiperiodic oscillation of a damped nonlinear system where the system is oscillatory even in absence of any external forcing. Our theoretical analysis of the parametric chemical oscillation is corroborated by full numerical simulation of two well known models of chemical dynamics, chlorite-iodine-malonic acid and iodine-clock reactions.

  10. Rayleigh-type parametric chemical oscillation.

    PubMed

    Ghosh, Shyamolina; Ray, Deb Shankar

    2015-09-28

    We consider a nonlinear chemical dynamical system of two phase space variables in a stable steady state. When the system is driven by a time-dependent sinusoidal forcing of a suitable scaling parameter at a frequency twice the output frequency and the strength of perturbation exceeds a threshold, the system undergoes sustained Rayleigh-type periodic oscillation, wellknown for parametric oscillation in pipe organs and distinct from the usual forced quasiperiodic oscillation of a damped nonlinear system where the system is oscillatory even in absence of any external forcing. Our theoretical analysis of the parametric chemical oscillation is corroborated by full numerical simulation of two well known models of chemical dynamics, chlorite-iodine-malonic acid and iodine-clock reactions.

  11. Rayleigh-type parametric chemical oscillation

    NASA Astrophysics Data System (ADS)

    Ghosh, Shyamolina; Ray, Deb Shankar

    2015-09-01

    We consider a nonlinear chemical dynamical system of two phase space variables in a stable steady state. When the system is driven by a time-dependent sinusoidal forcing of a suitable scaling parameter at a frequency twice the output frequency and the strength of perturbation exceeds a threshold, the system undergoes sustained Rayleigh-type periodic oscillation, wellknown for parametric oscillation in pipe organs and distinct from the usual forced quasiperiodic oscillation of a damped nonlinear system where the system is oscillatory even in absence of any external forcing. Our theoretical analysis of the parametric chemical oscillation is corroborated by full numerical simulation of two well known models of chemical dynamics, chlorite-iodine-malonic acid and iodine-clock reactions.

  12. Thermal radiation in Rayleigh-Benard instability

    NASA Astrophysics Data System (ADS)

    Lienhard, J. H.

    1990-02-01

    Thermal radiation from finite-conductivity boundaries can strongly affect the stability of horizontally unbounded plane fluid layers heated from below. The role of thermal radiation in plane-layer instabilities is studied under the assumption that the fluid medium is transparent (as a model of IR transfer through gas layers). The solution procedure modifies a previous formulation of the conductive boundary problem to account for the gray radiant interchange between boundaries. The nonisothermal character of the boundaries is shown to bias instability toward higher wavenumbers and to substantially increase the stability of fluid layers between radiative nonconductive boundaries relative to layers having nonradiative boundaries. A single layer is studied first, and then a case of parallel interacting fluid layers is considered. Critical Rayleigh numbers are presented as both tabulations and correlations. The implications for solar-collector design are discussed.

  13. Small Atwood number Rayleigh-Taylor experiments.

    PubMed

    Andrews, Malcolm J; Dalziel, Stuart B

    2010-04-13

    Consideration is given to small Atwood number (non-dimensional density difference) experiments to investigate mixing driven by Rayleigh-Taylor (R-T) instability. The past 20 years have seen the development of novel experiments to investigate R-T mixing and, simultaneously, the advent of high-fidelity diagnostics. Indeed, the developments of experiments and diagnostics have gone hand in hand, and as a result modern R-T experiments rival the capabilities and research scope of shear-driven mixing experiments. Thus, research into the small Atwood number limit has made significant progress over the past 20 years, and has offered important insights into natural mixing processes as well as the general R-T problem. This review of small Atwood number experiments serves as an opportunity to discuss progress, and also to provoke thoughts about future high Atwood number designs and difficulties.

  14. Anelastic Rayleigh-Taylor mixing layers

    NASA Astrophysics Data System (ADS)

    Schneider, N.; Gauthier, S.

    2016-07-01

    Anelastic Rayleigh-Taylor mixing layers for miscible fluids are investigated with a recently built model (Schneider and Gauthier 2015 J. Eng. Math. 92 55-71). Four Chebyshev-Fourier-Fourier direct numerical simulations are analyzed. They use different values for the compressibility parameters: Atwood number (the dimensionless difference of the heavy and light fluid densities) and stratification (accounts for the vertical variation of density due to gravity). For intermediate Atwood numbers and finite stratification, compressibility effects quickly occurs. As a result only nonlinear behaviours are reached. The influence of the compressibility parameters on the growth speed of the RTI is discussed. The 0.1—Atwood number/0.4—stratification configuration reaches a turbulent regime. This turbulent mixing layer is analyzed with statistical tools such as moments, PDFs, anisotropy indicators and spectra.

  15. Classical Rayleigh Taylor experiments on Nova

    SciTech Connect

    Budil, K.S.; Remington, B.A.; Peyser, T.A.

    1995-07-01

    The evolution of the Rayleigh-Taylor (RT) instability in a compressible medium was investigated both at an accelerating embedded interface and at the ablation front in a new series of experiments on Nova. The x-ray drive generated in a hohlraum ablatively accelerated a planar target consisting of a doped plastic pusher which was in some cases backed by a higher density titanium payload. Both target types were diagnosed by face-on and side-on radiography. Experiments have been done with a variety of wavelengths and initial amplitudes. In the case where the perturbed RT-unstable embedded interface is isolated from the ablation front, short wavelength perturbations are observed to grow strongly. When the perturbation is at the ablation front, the short wavelengths are observed to be severely stabilized.

  16. Effect of molecular anisotropy on the intensity and degree of polarization of light scattered from model atmospheres

    NASA Technical Reports Server (NTRS)

    Bahethi, O. P.; Fraser, R. S.

    1980-01-01

    Computations of the properties of sunlight scattered from models of the earth-atmosphere system are presented to show the effect of molecular anisotropy on the intensity, flux, and degree of polarization of the scattered light. The values of these parameters change significantly when the anisotropy factor is neglected in the molecular optical thickness and scattering phase matrix. However, if the Rayleigh scattering optical thickness is kept constant and the molecular anisotropy factor is included only in the Rayleigh phase matrix, the flux does not change, the intensity changes by a small amount, but the changes in the degree of polarization are still significant.

  17. Authentication of vegetable oils by confocal X-ray scattering analysis with coherent/incoherent scattered X-rays.

    PubMed

    Li, Fangzuo; Liu, Zhiguo; Sun, Tianxi

    2016-11-01

    This paper presents an alternative analytical method based on the Rayleigh to Compton scattering intensity ratio and effective atomic number for non-destructive identification of vegetable oils using confocal energy dispersive X-ray fluorescence and scattering spectrometry. A calibration curve for the Rayleigh to Compton scattering intensity ratio and effective atomic number was constructed on the basis of a reliable physical model for X-ray scattering. The content of light elements, which are "invisible" using X-ray fluorescence, can be calculated "by difference" from the calibration curve. In this work, we demonstrated the use of this proposed approach to identify complex organic matrices in different vegetable oils with high precision and accuracy.

  18. QUADRO: A SUPERVISED DIMENSION REDUCTION METHOD VIA RAYLEIGH QUOTIENT OPTIMIZATION.

    PubMed

    Fan, Jianqing; Ke, Zheng Tracy; Liu, Han; Xia, Lucy

    We propose a novel Rayleigh quotient based sparse quadratic dimension reduction method-named QUADRO (Quadratic Dimension Reduction via Rayleigh Optimization)-for analyzing high-dimensional data. Unlike in the linear setting where Rayleigh quotient optimization coincides with classification, these two problems are very different under nonlinear settings. In this paper, we clarify this difference and show that Rayleigh quotient optimization may be of independent scientific interests. One major challenge of Rayleigh quotient optimization is that the variance of quadratic statistics involves all fourth cross-moments of predictors, which are infeasible to compute for high-dimensional applications and may accumulate too many stochastic errors. This issue is resolved by considering a family of elliptical models. Moreover, for heavy-tail distributions, robust estimates of mean vectors and covariance matrices are employed to guarantee uniform convergence in estimating non-polynomially many parameters, even though only the fourth moments are assumed. Methodologically, QUADRO is based on elliptical models which allow us to formulate the Rayleigh quotient maximization as a convex optimization problem. Computationally, we propose an efficient linearized augmented Lagrangian method to solve the constrained optimization problem. Theoretically, we provide explicit rates of convergence in terms of Rayleigh quotient under both Gaussian and general elliptical models. Thorough numerical results on both synthetic and real datasets are also provided to back up our theoretical results.

  19. Brillouin scattering self-cancellation

    NASA Astrophysics Data System (ADS)

    Florez, O.; Jarschel, P. F.; Espinel, Y. A. V.; Cordeiro, C. M. B.; Mayer Alegre, T. P.; Wiederhecker, G. S.; Dainese, P.

    2016-06-01

    The interaction between light and acoustic phonons is strongly modified in sub-wavelength confinement, and has led to the demonstration and control of Brillouin scattering in photonic structures such as nano-scale optical waveguides and cavities. Besides the small optical mode volume, two physical mechanisms come into play simultaneously: a volume effect caused by the strain-induced refractive index perturbation (known as photo-elasticity), and a surface effect caused by the shift of the optical boundaries due to mechanical vibrations. As a result, proper material and structure engineering allows one to control each contribution individually. Here, we experimentally demonstrate the perfect cancellation of Brillouin scattering arising from Rayleigh acoustic waves by engineering a silica nanowire with exactly opposing photo-elastic and moving-boundary effects. This demonstration provides clear experimental evidence that the interplay between the two mechanisms is a promising tool to precisely control the photon-phonon interaction, enhancing or suppressing it.

  20. Brillouin scattering self-cancellation

    PubMed Central

    Florez, O.; Jarschel, P. F.; Espinel, Y. A. V.; Cordeiro, C. M. B.; Mayer Alegre, T. P.; Wiederhecker, G. S.; Dainese, P.

    2016-01-01

    The interaction between light and acoustic phonons is strongly modified in sub-wavelength confinement, and has led to the demonstration and control of Brillouin scattering in photonic structures such as nano-scale optical waveguides and cavities. Besides the small optical mode volume, two physical mechanisms come into play simultaneously: a volume effect caused by the strain-induced refractive index perturbation (known as photo-elasticity), and a surface effect caused by the shift of the optical boundaries due to mechanical vibrations. As a result, proper material and structure engineering allows one to control each contribution individually. Here, we experimentally demonstrate the perfect cancellation of Brillouin scattering arising from Rayleigh acoustic waves by engineering a silica nanowire with exactly opposing photo-elastic and moving-boundary effects. This demonstration provides clear experimental evidence that the interplay between the two mechanisms is a promising tool to precisely control the photon–phonon interaction, enhancing or suppressing it. PMID:27283092

  1. Laser Thomson scattering in a pulsed atmospheric arc discharge

    NASA Astrophysics Data System (ADS)

    Sommers, Bradley; Adams, Steven

    2015-09-01

    Laser scattering measurements, including Rayleigh, Raman, and Thomson scattering have been performed on an atmospheric pulsed arc discharge. Such laser scattering techniques offer a non-invasive diagnostic to measure gas temperature, electron temperature, and electron density in atmospheric plasma sources, particularly those with feature sizes approaching 1 mm. The pulsed discharge is ignited in a pin to pin electrode geometry using a 6 kV pulse with 10 ns duration. The electrodes are housed in a glass vacuum chamber filled with argon gas. The laser signal is produced by a Nd:Yag laser supply, repetitively pulsed at 10 Hz and frequency quadrupled to operate at 266 nm. The scattered laser signal is imaged onto a triple grating spectrometer, which is used to suppress the Rayleigh scatter signal in order to measure the low amplitude Thomson and Raman signals. Preliminary results include measurements of electron temperature and electron density in the plasma column taken during the evolution of the discharge. The laser system is also used to measure the Rayleigh scattering signal, which provides space and time resolved measurements of gas temperature in the arc discharge.

  2. Delinating Thermohaline Double-Diffusive Rayleigh Regimes

    NASA Astrophysics Data System (ADS)

    Graf, T.; Walther, M.; Kolditz, O.; Liedl, R.

    2013-12-01

    In natural systems, convective flow induced from density differences may occur in near-coastal aquifers, atmospheric boundary layers, oceanic streams or within the earth crust. Whether an initially stable, diffusive regime evolves into a convective (stable or chaotic) regime, or vice versa, depends on the system's framing boundary conditions. A conventional parameter to express the relation between diffusive and convective forces of such a density-driven regime is Rayleigh number (Ra). While most systems are mainly dominated by only a single significant driving force (i.e. only temperature or salinity), some systems need to consider two boundary processes (e.g. deep, thus warm, haline flow in porous media). In that case, a two-dimensional, 'double-diffusive' Rayleigh system can be defined. Nield (1998) postulated a boundary between diffusive and convective regime at RaT + RaC = 4pi^2 in the first quadrant (Q1), with Rayleigh numbers for temperature and concentration respectively. The boundary in the forth quadrant (Q4) could not exactly be determined, yet the approximate position estimated. Simulations with HydroGeoSphere (Therrien, 2010) using a vertical, quadratic, homogeneous, isotropic setup confirmed the existence of the 4pi^2-boundary and revealed additional regimes (diffusive, single-roll, double-roll, chaotic) in Q1. Also, non-chaotic, oscillating patterns could be identified in Q4. More detailed investigations with OpenGeoSys (Kolditz, 2012) confirmed the preceding HGS results, and, using a 1:10-scaled domain (height:length), uncovered even more distinctive regimes (diffusive, minimum ten roles, supposely up to 25 roles, and chaotic?) in Q1, while again, oscillating patterns were found in the transition zone between diffusive and chaotic regimes in Q4. Output of numerical simulations from Q1 and Q4 show the mentioned regimes (diffusive, stable-convective, stable-oscillatory, chaotic) while results are displayed in context of a possible delination between

  3. Short Rayleigh length free electron laser: Experiments and simulations

    SciTech Connect

    Crooker, P.P.; Colson, William; Blau, Joe; Burggraff, D.; Sans Aguilar, J.; Benson, Stephen; Neil, George; Michelle D. Shinn; Evtushenko, Pavel

    2008-09-01

    DOI: http://dx.doi.org/10.1103/PhysRevSTAB.11.090701
    We report experiments at Jefferson National Accelerator Facility (Jlab) and computer simulations performed at the Naval Postgraduate School (NPS) designed to probe the small Rayleigh length regime. We compare the gain, power, and sensitivity to mirror and electron beam misalignments as a function of decreasing Rayleigh length. The agreement is quite good, with experiments and simulations showing comparable trends as the Rayleigh length is decreased. In particular, we find that the gain and power do not decrease substantially at short Rayleigh length, contrary to a common Gaussian-mode filling factor argument. Within currently achievable alignment tolerances, the gain and power are still acceptable for FEL operation.

  4. Generalized Rayleigh and Jacobi Processes and Exceptional Orthogonal Polynomials

    NASA Astrophysics Data System (ADS)

    Chou, C.-I.; Ho, C.-L.

    2013-09-01

    We present four types of infinitely many exactly solvable Fokker-Planck equations, which are related to the newly discovered exceptional orthogonal polynomials. They represent the deformed versions of the Rayleigh process and the Jacobi process.

  5. Beating Rayleigh's Curse by Imaging Using Phase Information.

    PubMed

    Tham, Weng-Kian; Ferretti, Hugo; Steinberg, Aephraim M

    2017-02-17

    Every imaging system has a resolution limit, typically defined by Rayleigh's criterion. Given a fixed number of photons, the amount of information one can gain from an image about the separation between two sources falls to zero as the separation drops below this limit, an effect dubbed "Rayleigh's curse." Recently, in a quantum-information-inspired proposal, Tsang and co-workers found that there is, in principle, infinitely more information present in the full electromagnetic field in the image plane than in the intensity alone, and suggested methods for extracting this information and beating the Rayleigh limit. In this Letter, we experimentally demonstrate a simple scheme that captures most of this information, and show that it has a greatly improved ability to estimate the distance between a pair of closely separated sources, achieving near-quantum-limited performance and immunity to Rayleigh's curse.

  6. Beating Rayleigh's Curse by Imaging Using Phase Information

    NASA Astrophysics Data System (ADS)

    Tham, Weng-Kian; Ferretti, Hugo; Steinberg, Aephraim M.

    2017-02-01

    Every imaging system has a resolution limit, typically defined by Rayleigh's criterion. Given a fixed number of photons, the amount of information one can gain from an image about the separation between two sources falls to zero as the separation drops below this limit, an effect dubbed "Rayleigh's curse." Recently, in a quantum-information-inspired proposal, Tsang and co-workers found that there is, in principle, infinitely more information present in the full electromagnetic field in the image plane than in the intensity alone, and suggested methods for extracting this information and beating the Rayleigh limit. In this Letter, we experimentally demonstrate a simple scheme that captures most of this information, and show that it has a greatly improved ability to estimate the distance between a pair of closely separated sources, achieving near-quantum-limited performance and immunity to Rayleigh's curse.

  7. Rayleigh-Lagrange formalism for classical dissipative systems.

    PubMed

    Virga, Epifanio G

    2015-01-01

    It is often believed that the Rayleigh-Lagrange formalism for classical dissipative systems is unable to encompass forces described by nonlinear functions of the velocities. Here we show that this is indeed a misconception.

  8. Linear instability in Rayleigh-stable Taylor-Couette flow

    NASA Astrophysics Data System (ADS)

    Deguchi, Kengo

    2017-02-01

    Rayleigh's stability criterion describes the inviscid stability of rotating fluid flows. Despite the limitations of the criterion due to the assumptions used, it has been widely viewed as a general stability barrier in various rapidly rotating flows. However, contrary to previous belief, a linear instability is identified in Rayleigh-stable Taylor-Couette flow. The instability is found in cyclonic rapid rotation regime, for almost the entire range of the radius ratio of the cylinders.

  9. Suppression of Rayleigh Taylor instability in strongly coupled plasmas

    SciTech Connect

    Das, Amita; Kaw, Predhiman

    2014-06-15

    The Rayleigh Taylor instability in a strongly coupled plasma medium has been investigated using the equations of generalized hydrodynamics. It is demonstrated that the visco-elasticity of the strongly coupled medium due to strong inter particle correlations leads to a suppression of the Rayleigh Taylor instability unless certain threshold conditions are met. The relevance of these results to experiments on laser compression of matter to high densities including those related to inertial confinement fusion using lasers has also been shown.

  10. Phase turbulence in rayleigh-Benard convection

    PubMed

    Xi; Li; Gunton

    2000-12-01

    We present a three-dimensional simulation of Rayleigh-Benard convection in a large aspect ratio Gamma=60 with stress-free boundaries for a fluid Prandtl number sigma=0.5. We find that a spatiotemporal chaotic state (phase turbulence) emerges immediately above onset, which we investigate as a function of the reduced control parameter epsilon. In particular we find that the correlation length for the vertical velocity field, the time averaged convective current, and the mean square vorticity have power law behaviors near onset, with exponents given by -1/2, 1, and 5/2 respectively. We also find that the time averaged vertical velocity and vertical vorticity fields have the same (disordered) spatial characteristics as the corresponding instantaneous patterns for these fields, and that there is no long-term phase correlation in the system. Finally, we present simple theoretical explanations for the time averaged convective current as a function of the control parameter, and for the fact that the time dependence of three global quantities (characterizing the dissipation of kinetic energy, the release of internal energy by buoyancy, and entropy flow) is essentially the same.

  11. Range of validity of the Rayleigh hypothesis.

    PubMed

    Watanabe, T; Choyal, Y; Minami, K; Granatstein, V L

    2004-05-01

    The parameter range over which the Rayleigh hypothesis (RH) for optical gratings might be validly applied to analysis of high power backward wave oscillators has been investigated numerically. It had been pointed out that from a rigorous mathematical viewpoint, RH was only valid for a shallow corrugation of slow wave structure (SWS) such that h K0 <0.448; here, h and K0 are, respectively, the amplitude and wave number of the periodicity in a sinusoidal planar grating. We numerically analyze the electromagnetic fields in the axisymmetric SWS with and without use of RH. The field patterns and eigenfrequency for the SWS are solved numerically for a given k(z) by using the code HIDM (higher order implicit difference method) that is free from the RH. It is found that, for a deep corrugation, h K0 =5 x 0.448, using RH is still valid for obtaining the dispersion relation, although the Floquet harmonic expansion (FHE) fails to correctly represent the field patterns inside the corrugation. Accordingly, there exists a discrepancy between the validity of using RH for obtaining dispersion relations and for an exact convergence of FHE everywhere in the SWS.

  12. Energy transfer in Rayleigh-Taylor instability.

    PubMed

    Cook, Andrew W; Zhou, Ye

    2002-08-01

    The spatial structure and energy budget for Rayleigh-Taylor instability are examined using results from a 512 x 512 x 2040 point direct numerical simulation. The outer-scale Reynolds number of the flow follows a rough t(3) power law and reaches a final value of about 5500. Taylor microscales and Reynolds numbers are plotted to characterize anisotropy in the flow and document progress towards the mixing transition. A mixing parameter is defined which characterizes the relative rates of entrainment and mixing in the flow. The spectrum of each term in the kinetic energy equation is plotted, at regular time intervals, as a function of the inhomogeneous direction and the two-dimensional wave number for the homogeneous directions. The energy spectrum manifests the beginning of an inertial range by the latter stages of the simulation. The production and dissipation spectra become increasingly opposite and separate in wave space as the flow evolves. The transfer spectrum depends strongly on the inhomogeneous direction, with the net transfer being from large to small scales. Energy transfer at the bubble/spike fronts is strictly positive. Extensive cancellation occurs between the pressure and advection terms. The dilatation term produces negligible energy transfer, but its overall effect is to move energy from high to low density regions.

  13. Rayleigh-Taylor instability simulations with CRASH

    NASA Astrophysics Data System (ADS)

    Chou, C.-C.; Fryxell, B.; Drake, R. P.

    2012-03-01

    CRASH is a code package developed for the predictive study of radiative shocks. It is based on the BATSRUS MHD code used extensively for space-weather research. We desire to extend the applications of this code to the study of hydrodynamically unstable systems. We report here the results of Rayleigh-Taylor instability (RTI) simulations with CRASH, as a necessary step toward the study of such systems. Our goal, motivated by the previous comparison of simulations and experiment, is to be able to simulate the magnetic RTI with self-generated magnetic fields produced by the Biermann Battery effect. Here we show results for hydrodynamic RTI, comparing the effects of different solvers and numerical parameters. We find that the early-time behavior converges to the analytical result of the linear theory. We observe that the late-time morphology is sensitive to the numerical scheme and limiter beta. At low-resolution limit, the growth of RTI is highly dependent on the setup and resolution, which we attribute to the large numerical viscosity at low resolution.

  14. Non-adiabatic Rayleigh-Taylor instability

    NASA Astrophysics Data System (ADS)

    Canfield, Jesse; Denissen, Nicholas; Reisner, Jon

    2016-11-01

    Onset of Rayleigh-Taylor instability (RTI) in a non-adiabatic environment is investigated with the multi-physics numerical model, FLAG. This work was inspired by laboratory experiments of non-adiabatic RTI, where a glass vessel with a layer of tetrahyrdofuran (THF) below a layer of toluene was placed inside a microwave. THF, a polar solvent, readily absorbs electromagnetic energy from microwaves. Toluene, a non-polar solvent, is nearly transparent to microwave heating. The presence of a heat source in the THF layer produced convection and a time-dependent Atwood number (At). The system, initially in stable hydrostatic equilibrium At < 0 , was set into motion by microwave induced, volumetric heating of the THF. The point when At > 0 , indicates that the system is RTI unstable. The observed dominant mode at the onset of RTI was the horizontal length scale of the vessel. This scale is contrary to classical RTI, where the modes start small and increases in scale with time. It is shown that the dominant RTI mode observed in the experiments was determined by the THF length scale prior to RTI. The dominant length scale transitions from the THF to the toluene via the updrafts and downdrafts in the convective cells. This happens when At passes from negative to positive. This work was funded by the Advanced Simulation and Computing Program.

  15. A Comparison of Short Rayleigh Range FEL Performance with Simulations

    SciTech Connect

    Benson, Stephen; Evtushenko, Pavel; Michelle D. Shinn; Neil, George; Blau, Joe; Burggraff, D.; Colson, William; Crooker, P.P.; Sans Aguilar, J.

    2007-08-01

    One approach to attaining very high power in a free-electron laser (FEL) is to operate with a Rayleigh range much smaller than the wiggler length. Previously, 3D simulations of Free-electron laser (FEL) oscillators showed that FEL gain doesn't fall off with Rayleigh range as predicted by one-dimensional simulations*. They also predict that the angular tolerance for the mirrors is much large than simplistic theory predicts. Using the IR Upgrade laser at Jefferson Lab lasing at 935 nm we have studied the performance of an FEL with very short Rayleigh range. We also looked at the angular sensitivity for several different Rayleigh ranges. We find very good agreement between simulations and measured gain and angular sensitivities. Surprisingly the gain continues to rise as the Rayleigh range is shortened and continues to grow even when the resonator becomes geometrically unstable. The same behavior is seen in both the experiment and simulations. We also find that, even for large Rayleigh r

  16. Power coupling characteristics between FBG and back-scattering signals

    NASA Astrophysics Data System (ADS)

    Li, Jianzhi; Zhao, Desheng; Hou, Yuemin; Sun, Baochen

    2017-03-01

    The property and compatibility between fiber Bragg grating (FBG) and back-scattering signals are investigated by employing optical time domain reflectometry. We compare the power spectrums of spontaneous Brillouin scattering (SpBS), simultaneous Brillouin scattering (SBS) and Rayleigh scattering (RS), and coupling mechanism between FBG and back-scattering signal is explored. Experimental results show that the region of FBG contributes to the backscatter power and causes the desired reflection, and the power peak of FBG in SBS power spectrum is the sharpest among back-scattering light power spectrums and broadens with the decrease of spatial resolution. Moreover, the FBG-based method is used to find the location of temperature or stain event for scatter-based distributed sensors.

  17. Non-coherent Continuum Scattering as a Line Polarization Mechanism

    NASA Astrophysics Data System (ADS)

    del Pino Alemán, T.; Manso Sainz, R.; Trujillo Bueno, J.

    2014-03-01

    Line scattering polarization can be strongly affected by Rayleigh scattering at neutral hydrogen and Thomson scattering at free electrons. Often a depolarization of the continuum results, but the Doppler redistribution produced by the continuum scatterers, which are light (hence, fast), induces more complex interactions between the polarization in spectral lines and in the continuum. Here we formulate and solve the radiative transfer problem of scattering line polarization with non-coherent continuum scattering consistently. The problem is formulated within the spherical tensor representation of atomic and light polarization. The numerical method of solution is a generalization of the Accelerated Lambda Iteration that is applied to both the atomic system and the radiation field. We show that the redistribution of the spectral line radiation due to the non-coherence of the continuum scattering may modify the shape of the emergent fractional linear polarization patterns significantly, even yielding polarization signals above the continuum level in intrinsically unpolarizable lines.

  18. Effects of elastic focusing on global models of Rayleigh wave attenuation

    NASA Astrophysics Data System (ADS)

    Bao, Xueyang; Dalton, Colleen A.; Ritsema, Jeroen

    2016-11-01

    Rayleigh wave amplitudes are the primary data set used for imaging shear attenuation in the upper mantle on a global scale. In addition to attenuation, surface-wave amplitudes are influenced by excitation at the earthquake source, focusing and scattering by elastic heterogeneity, and local structure at the receiver and the instrument response. The challenge of isolating the signal of attenuation from these other effects limits both the resolution of global attenuation models and the level of consistency between different global attenuation studies. While the source and receiver terms can be estimated using relatively simple approaches, focusing effects on amplitude are a large component of the amplitude signal and are sensitive to multiscale velocity anomalies. In this study we investigate how different theoretical treatments for focusing effects on Rayleigh wave amplitude influence the retrieved attenuation models. A new data set of fundamental-mode Rayleigh wave phase and amplitude at periods of 50 and 100 sis analysed. The amplitudes due to focusing effects are predicted using the great-circle ray approximation (GCRA), exact ray theory (ERT), and finite-frequency theory (FFT). Phase-velocity maps expanded to spherical-harmonic degree 20 and degree 40 are used for the predictions. After correction for focusing effects, the amplitude data are inverted for global attenuation maps and frequency-dependent source and receiver correction factors. The degree-12 attenuation maps, based on different corrections for focusing effects, all contain the same large-scale features, though the magnitude of the attenuation variations depends on the focusing correction. The variance reduction of the amplitudes strongly depends on the predicted focusing amplitudes, with the highest variance reduction for the ray-based approaches at 50 s and for FFT at 100 s. Although failure to account for focusing effects introduces artefacts into the attenuation models at higher spherical

  19. Discrete ordinate theory of radiative transfer. 2: Scattering from maritime haze

    NASA Technical Reports Server (NTRS)

    Kattawar, G. W.; Plass, G. N.; Catchings, F. E.

    1971-01-01

    Discrete ordinate theory was used to calculate the reflected and transmitted radiance of photons which have interacted with plane parallel maritime haze layers. The results are presented for three solar zenith angles, three values of the surface albedo, and a range of optical thicknesses from very thin to very thick. The diffuse flux at the lower boundary and the cloud albedo were tabulated. The forward peak and other features in the single scattered phase function caused the radiance in many cases to be very different from that for Rayleigh scattering. The variation of the radiance with both the zenith or nadir angle and the azimuthal angle is more marked, and the relative limb darkening under very thick layers is greater, for haze than for Rayleigh scattering. The downward diffuse flux at the lower boundary for A = O is always greater and the cloud albedo is always less for haze than for Rayleigh layers.

  20. Aluminum Rayleigh Taylor Strength Measurements and Calculations

    SciTech Connect

    Lindquist, M J; Cavallo, R M; Lorenz, K T; Pollaine, S M; Remington, B A; Raevsky, V A

    2007-01-10

    A traditional approach to the study of material strength has been revitalized at the Russian Federal Nuclear Center (VNIIEF). Rayleigh Taylor strength experiments have long been utilized to measure the material response of metals at high pressure and strain rates. A modulated (sinusoidal or sawtooth perturbation) surface is shocklessly (quasi-isentropically) accelerated by a high explosive (HE) driver, and radiography is used to measure the perturbation amplitude as a function of time. The Aluminum T-6061 targets are designed with several sets of two-dimensional sawtooth perturbations machined on the loading surface. The HE driver was designed to reach peak pressures in the range of 200 to 300 kbar and strain rates in the range of 10{sup 4} - 10{sup 6} s{sup -1}. The standard constitutive strength models, Steinberg-Guinan (SG) [1], Steinberg-Lund (SL) [2], Preston-Tonks-Wallace (PTW) [3], Johnson-Cooke (JC) [4], and Mechanical Threshold Stress (MTS) [5], have been calibrated by traditional techniques: (Hopkinson-Bar, Taylor impact, flyer plate/shock-driven experiments). The VNIIEF experimental series accesses a strain rate regime not attainable using traditional methods. We have performed a detailed numerical study with a two-dimensional Arbitrary Lagrangian Eulerian hydrodynamics computer code containing several constitutive strength models to predict the perturbation growth. Results show that the capabilities of the computational methodology predict the amplitude growth to within 5 percent of the measured data, thus validating both the code and the strength models under the given conditions and setting the stage for credible future design work using different materials.

  1. New directions for Rayleigh-Taylor mixing.

    PubMed

    Glimm, James; Sharp, David H; Kaman, Tulin; Lim, Hyunkyung

    2013-11-28

    We study the Rayleigh-Taylor (RT) mixing layer, presenting simulations in agreement with experimental data. This problem is an idealized subproblem of important scientific and engineering problems, such as gravitationally induced mixing in oceanography and performance assessment for inertial confinement fusion. Engineering codes commonly achieve correct simulations through the calibration of adjustable parameters. In this sense, they are interpolative and not predictive. As computational science moves from the interpolative to the predictive and reduces the reliance on experiment, the quality of decision making improves. The diagnosis of errors in a multi-parameter, multi-physics setting is daunting, so we address this issue in the proposed idealized setting. The validation tests presented are thus a test for engineering codes, when used for complex problems containing RT features. The RT growth rate, characterized by a dimensionless but non-universal parameter α, describes the outer edge of the mixing zone. Increasingly accurate front tracking/large eddy simulations reveal the non-universality of the growth rate and agreement with experimental data. Increased mesh resolution allows reduction in the role of key subgrid models. We study the effect of long-wavelength perturbations on the mixing growth rate. A self-similar power law for the initial perturbation amplitudes is here inferred from experimental data. We show a maximum ±5% effect on the growth rate. Large (factors of 2) effects, as predicted in some models and many simulations, are inconsistent with the experimental data of Youngs and co-authors. The inconsistency of the model lies in the treatment of the dynamics of bubbles, which are the shortest-wavelength modes for this problem. An alternative theory for this shortest wavelength, based on the bubble merger model, was previously shown to be consistent with experimental data.

  2. Performance evaluation of a dual fringe-imaging Michelson interferometer for air parameter measurements with a 355 nm Rayleigh-Mie lidar.

    PubMed

    Cézard, Nicolas; Dolfi-Bouteyre, Agnès; Huignard, Jean-Pierre; Flamant, Pierre H

    2009-04-20

    A new concept of spectrum analyzer is proposed for short-range lidar measurements in airborne applications. It implements a combination of two fringe-imaging Michelson interferometers to analyze the Rayleigh-Mie spectrum backscattered by molecules and particles at 355 nm. The objective is to perform simultaneous measurements of four variables: the air speed, the air temperature and density, and the particle scattering ratio. The Cramer-Rao bounds are calculated to evaluate the best expectable measurement accuracies. The performance optimization shows that a Michelson interferometer with a path difference of 3 cm is optimal for air speed measurements in clear air. To optimize density, temperature, and scattering ratio measurements, the second interferometer should be set to a path difference of 10 cm at least; 20 cm would be better to be less sensitive to the actual Rayleigh-Brillouin line shape.

  3. Sub-one-nanometer gap (SONG) for nanogap-enhanced Raman scattering (NERS)

    NASA Astrophysics Data System (ADS)

    Lee, Haemi; Lee, Jung-Hoon; Nam, Jwa-Min; Suh, Yung Doug

    2016-09-01

    Accurate measurement of Rayleigh scattering is crucially important for fundamental understanding of the plasmonic properties of meltimeric (>= 3) nanoparticles that can be served as efficient SERS sensing platforms and nanophotonic materials. Thus, using the laser-scanning assisted dark-field microscopy that enabled to precisely collect far-field (Rayleigh) scattering from the centers of individual trimeric nanoparticles, we monitored spectral redistributions of oscillating coupled plasmonic modes as a function of trimer symmetry. As a consequence of the precise measurement of the polarization-resolved Rayleigh scattering spectra obtained from triangular trimers to linear trimers via elongated triangular trimers, the in-phase horizontally oscillating plasmonic mode with the largest dipole moment is found to be greatly increased by 20-folds, whereas the axially oscillating plasmonic mode with the second-largest dipole moment is dramatically decreased by 70-folds. Consequently, the overall quantity of the far-field scattering, the total sum of the individual coupled plasmonic modes, was gradually increased by 2-folds. The precise polarization-resolved Rayleigh scattering measurement also visualizes directly the directions of the radiation fields of individual oscillating coupled plasmonic modes, which would be valuable information in systematic controlling the polarization direction of the scattered light from the trimers. Overall, we showed an exemplary quantitative and extensive study of the coupled plasmonic modes from nanoparticles, giving a simple but clear insight.

  4. Lithospheric imaging via teleseismic scattering tomography

    NASA Astrophysics Data System (ADS)

    Frederiksen, A. W.; Revenaugh, J.

    2004-12-01

    The coda of the teleseismic P phase consists largely of energy scattered by small inhomogeneities in the receiver-side lithosphere. Given large collections of teleseismic data from dense permanent networks, previous workers have successfully back-propagated coda energy back to scattering source points using various kinematic migration schemes, as well as by inverting using an inverse scattering/radon transform approach. Under the Born approximation, seismic scattering is a linear process; therefore it is possible to approach coda scattering as a linear waveform inversion problem, mathematically similar to transmission-based tomography. Assuming ray-theoretical propagation and Rayleigh scattering, we pose the inverse scattering problem in tomographic form, and recover perturbations in density and P and S velocities from Pp and Ps scattered data. The method is applied to data from the Southern California Seismic Network (SCSN) covering the San Jacinto-Anza region. The results show a considerable correlation between seismicity and velocity perturbation structure, particularly in the region between the Mission Creek and Banning fault branches. Features connecting the Coyote Creek and Elsinore faults at right angles are correlated with seismicity lineations and may represent conjugate faulting with no surface expression.

  5. Light scattering by a thin wire with a surface-plasmon resonance: Bifurcations of the Poynting vector field

    SciTech Connect

    Luk'yanchuk, B. S.; Ternovsky, V.

    2006-06-15

    We analyze the energy flow during the scattering of a plane wave by a small homogeneous cylinder in the vicinity of surface-plasmon resonance, where {epsilon}{sup '}=Re {epsilon}=-1 ({epsilon} stands for permittivity). For the case of small dissipation, {epsilon}{sup ''}=Im {epsilon}<<1, this scattering can strongly deviate from the classical dipole approximation (Rayleigh scattering). In certain specified cases, the Rayleigh scattering is replaced with an anomalous light scattering regardless the wire smallness. The phenomenon is based on interplay of the usual dissipative and radiative damping, where the latter is related to inverse transformation of localized resonant plasmons into scattered light. The anomalous light scattering possesses a variety of unusual features, such as an inverse hierarchy of optical resonances and a complicated near-field structure, which may include optical vortexes, optical whirlpools, and other peculiarities in nanoscale area.

  6. Scattering of guided light by a single hole in a dielectric slab.

    PubMed

    Mariani, F; van Exter, M P

    2015-06-29

    We study the scattering of waveguided light by a single hole in a dielectric slab with FDTD simulations and investigate two scattering processes: two dimensional (2D) scattering into slab modes and three-dimensional (3D) scattering into the surroundings. We find that 2D scattering typically dominates over the 3D losses. We find important quantitative differences between the single hole scattering and the case of scattering from an infinite Mie cylinder. Additionally, we find that a hole cannot be simply modelled as a dipolar object even in the limit of small scatterers (Rayleigh approximation). This is visible from the angular dependence of the 2D scattered intensity. We discuss the relevance of our findings in the modeling of two dimensional random scattering media.

  7. Early Temperatures Observed with the Extremely Sensitive Rayleigh Lidar at Utah State University

    NASA Astrophysics Data System (ADS)

    Wickwar, Vincent B.; Sox, Leda; Emerick, Matthew T.; Herron, Joshua P.; Barton, David L.

    2016-06-01

    Rayleigh-scatter lidar observations were made at the Atmospheric Lidar Observatory (ALO) at Utah State University (USU) from 1993-2004 from 45-90 km. The lidar operated at 532 nm with a power-aperture-product (PAP) of ~3.1 Wm2. The sensitivity of the lidar has since been increased by a factor of 66 to 205 Wm2, extending the maximum altitude into new territory, the lower thermosphere. Observations have been extended up to 115 km, almost to the 120 km goal. Early temperatures from four ~4-week periods starting in June 2014 are presented and discussed. They are compared to each other, to the ALO climatology from the original lidar [1], and to temperatures from the NRLMSISe00 empirical model [2].

  8. The interconnection of degree of coherence and Rayleigh particles velocity motion

    NASA Astrophysics Data System (ADS)

    Soltys, I. V.

    2016-09-01

    The proposed paper investigates the influence of a coherence degree of superposing mutually orthogonal linearly-polarized waves on the peculiarities of nanosize range particle motion in the inhomogeneously polarized optical field and field of the averaged values of the Poynting vector. In this case the depth of the energy volume density modulation essentially depends on the degree of coherence of interacting waves. The way of monitoring particles of the Rayleigh light scattering mechanism in the energy inhomogeneous optical field is proposed for investigation. The increase of spin flows influence on optical fields studying is analyzed. The possibility of controlling particles of different properties and characteristics becomes possible due to the intrinsic optical flows action.

  9. Photon Scattering in 3D Radiative MHD Simulations

    NASA Astrophysics Data System (ADS)

    Hayek, Wolfgang

    2009-09-01

    Recent results from 3D time-dependent radiative hydrodynamic simulations of stellar atmospheres are presented, which include the effects of coherent scattering in the radiative transfer treatment. Rayleigh scattering and electron scattering are accounted for in the source function, requiring an iterative solution of the transfer equation. Opacities and scattering coefficients are treated in the multigroup opacity approximation. The impact of scattering on the horizontal mean temperature structure is investigated, which is an important diagnostic for model atmospheres, with implications for line formation and stellar abundance measurements. We find that continuum scattering is not important for the atmosphere of a metal-poor Sun with metailicity [Fe/H] = -3.0, similar to the previously investigated photosphere at solar metallicity.

  10. Modelling of microwave emission and scattering from snow and soil

    NASA Technical Reports Server (NTRS)

    Fung, Adrian K.; Chen, M. F.

    1989-01-01

    In the past a snow layer has been modeled as a homogeneous layer embedded with sparsely populated Rayleigh scatterers above an irregular ground surface. The effect of the ground surface can be ignored if the layer is sufficiently lossy due to wetness in the snow. The top surface of the snow layer may be treated as plane or irregular depending upon its actual shape and its wetness condition. For a dry snow condition where the electromagnetic wave can penetrate easily one can ignore the air-snow interface. As a result a variety of emission and scattering models exist. An improvement to the existing scattering or emission model would consist of an irregular layer with densely populated correlated scatterers. The development of this model and its application to scattering and emission from a snow layer are discussed. Also disucssed is a surface scattering model for a soil surface.

  11. Efficiencies of Rotational Raman, and Rayleigh Techniques for Laser Remote Sensing of the Atmospheric Temperature

    NASA Technical Reports Server (NTRS)

    Ivanova, I. D.; Gurdev, L. L.; Mitev, V. M.

    1992-01-01

    Various lidar methods have been developed for measuring the atmospheric temperature, making use of the temperature dependant characteristics of rotational Raman scattering (RRS) from nitrogen and oxygen, and Rayleigh or Rayleigh-Brillowin scattering (RS or RBS). These methods have various advantages and disadvantages as compared to each other but their potential accuracies are principal characteristics of their efficiency. No systematic attempt has been undertaken so far to compare the efficiences, in the above meaning, of different temperature lidar methods. Two RRS techniques have been compared. Here, we do such a comparison using two methods based on the detection and analysis of RS (RBS) spectra. Four methods are considered here for measuring the atmospheric temperature. One of them (Schwiesow and Lading, 1981) is based on an analysis of the RS linewidth with two Michelson interferometers (MI) in parallel. The second method (Shimisu et al., 1986) employs a high-resolution analysis of the RBS line shape. The third method (Cooney, 1972) employs the temperature dependance of the RRS spectrum envelope. The fourth method (Armstrong, 1974) makes use of a scanning Fabry-Perot interferometer (FPI) as a comb filter for processing the periodic RRS spectrum of the nitrogen. Let us denote the corresponding errors in measuring the temperature by sigma(sub MI), sigma(sub HR), sigma(sub ENV), and sigma(sub FPI). Let us also define the ratios chi(sub 1) = sigma(sub MI)/sigma(sub ENV), chi(sub 2) = sigma(sub HR)/sigma(sub ENV), and chi(sub 3) = sigma(sub FPI)/sigma(sub ENV) interpreted as relative errors with respect to sigma(sub ENV).

  12. Rayleigh-Taylor instability of violently collapsing bubbles

    NASA Astrophysics Data System (ADS)

    Lin, Hao; Storey, Brian D.; Szeri, Andrew J.

    2002-08-01

    In a classical paper Plesset has determined conditions under which a bubble changing in volume maintains a spherical shape. The stability analysis was further developed by Prosperetti to include the effects of liquid viscosity on the evolving shape modes. In the present work the theory is further modified to include the changing density of the bubble contents. The latter is found to be important in violent collapses where the densities of the gas and vapor within a bubble may approach densities of the liquid outside. This exerts a stabilizing influence on the Rayleigh-Taylor mechanism of shape instability of spherical bubbles. A comparison with experimental data shows good agreement with the new theory; the Rayleigh-Taylor instability does provide an extinction threshold for violently collapsing bubbles. It is also explained why earlier works did not produce a slope in the Rayleigh-Taylor stability curve that conforms with that of the present work.

  13. Bounded Rayleigh mixture model for ultrasound image segmentation

    NASA Astrophysics Data System (ADS)

    Bi, H.; Tang, H.; Shu, H. Z.; Dillenseger, J. L.

    2017-02-01

    The finite mixture model based on the Gaussian distribution is a flexible and powerful tool to address image segmentation. However, in the case of ultrasound images, the intensity distributions are non-symmetric whereas the Gaussian distribution is symmetric. In this study, a new finite bounded Rayleigh distribution is proposed. One advantage of the proposed model is that Rayleigh distribution is non-symmetric which has ability to fit the shape of medical ultrasound data. Another advantage is that each component of the proposed model is suitable for the ultrasound image segmentation. We also apply the bounded Rayleigh mixture model in order to improve the accuracy and to reduce the computational time. Experiments show that the proposed model outperforms the state-of-art methods on time consumption and accuracy.

  14. Modeling SAR images with a generalization of the Rayleigh distribution.

    PubMed

    Kuruoğlu, Ercan E; Zerubia, Josiane

    2004-04-01

    Synthetic aperture radar (SAR) imagery has found important applications due to its clear advantages over optical satellite imagery one of them being able to operate in various weather conditions. However, due to the physics of the radar imaging process, SAR images contain unwanted artifacts in the form of a granular look which is called speckle. The assumptions of the classical SAR image generation model lead to a Rayleigh distribution model for the histogram of the SAR image. However, some experimental data such as images of urban areas show impulsive characteristics that correspond to underlying heavy-tailed distributions, which are clearly non-Rayleigh. Some alternative distributions have been suggested such as the Weibull, log-normal, and the k-distribution which had success in varying degrees depending on the application. Recently, an alternative model namely the alpha-stable distribution has been suggested for modeling radar clutter. In this paper, we show that the amplitude distribution of the complex wave, the real and the imaginery components of which are assumed to be distributed by the alpha-stable distribution, is a generalization of the Rayleigh distribution. We demonstrate that the amplitude distribution is a mixture of Rayleighs as is the k-distribution in accordance with earlier work on modeling SAR images which showed that almost all successful SAR image models could be expressed as mixtures of Rayleighs. We also present parameter estimation techniques based on negative order moments for the new model. Finally, we test the performance of the model on urban images and compare with other models such as Rayleigh, Weibull, and the k-distribution.

  15. Study on evaluation methods for Rayleigh wave dispersion characteristic

    USGS Publications Warehouse

    Shi, L.; Tao, X.; Kayen, R.; Shi, H.; Yan, S.

    2005-01-01

    The evaluation of Rayleigh wave dispersion characteristic is the key step for detecting S-wave velocity structure. By comparing the dispersion curves directly with the spectra analysis of surface waves (SASW) method, rather than comparing the S-wave velocity structure, the validity and precision of microtremor-array method (MAM) can be evaluated more objectively. The results from the China - US joint surface wave investigation in 26 sites in Tangshan, China, show that the MAM has the same precision with SASW method in 83% of the 26 sites. The MAM is valid for Rayleigh wave dispersion characteristic testing and has great application potentiality for site S-wave velocity structure detection.

  16. Rotating Rayleigh-Benard convection: The Kueppers-Lortz transition

    SciTech Connect

    Zhong, F.; Ecke, R.; Steinberg, V.

    1990-01-01

    Rayleigh-Benard convection with rotation about a vertical axis is investigated for small dimensionless rotation rates 0 < {Omega} < 50. The convection cell is cylindrical with aspect ratio {Gamma} = 10 and the convecting fluid is water with a Prandtl number of 6.8 at T = 23.8C. Comparisons are made between experimental data and linear stability theory for the onset Rayleigh number and for the wave number dependence of the convective pattern. The nonlinear Kueppers-Lortz transition is found to occur significantly below the theoretically expected rotation rate {Omega}{sub c} and to be nucleated by defects created at the lateral cell walls. 20 refs., 10 figs.

  17. Covariant Lyapunov vectors of chaotic Rayleigh-Bénard convection

    NASA Astrophysics Data System (ADS)

    Xu, M.; Paul, M. R.

    2016-06-01

    We explore numerically the high-dimensional spatiotemporal chaos of Rayleigh-Bénard convection using covariant Lyapunov vectors. We integrate the three-dimensional and time-dependent Boussinesq equations for a convection layer in a shallow square box geometry with an aspect ratio of 16 for very long times and for a range of Rayleigh numbers. We simultaneously integrate many copies of the tangent space equations in order to compute the covariant Lyapunov vectors. The dynamics explored has fractal dimensions of 20 ≲Dλ≲50 , and we compute on the order of 150 covariant Lyapunov vectors. We use the covariant Lyapunov vectors to quantify the degree of hyperbolicity of the dynamics and the degree of Oseledets splitting and to explore the temporal and spatial dynamics of the Lyapunov vectors. Our results indicate that the chaotic dynamics of Rayleigh-Bénard convection is nonhyperbolic for all of the Rayleigh numbers we have explored. Our results yield that the entire spectrum of covariant Lyapunov vectors that we have computed are tangled as indicated by near tangencies with neighboring vectors. A closer look at the spatiotemporal features of the Lyapunov vectors suggests contributions from structures at two different length scales with differing amounts of localization.

  18. Regionalized Rayleigh wave group velocities in southeastern Brazil

    NASA Astrophysics Data System (ADS)

    Souza, J. L.; Dos Santos, N. P.; Pacheco, R. P.

    2003-04-01

    Damped least-square inversion was used to regionalize a large quantity of source-station Rayleigh wave dispersion curves obtained from digital seismograms, which were recorded at twenty-three IRIS seismological stations located either in or around South America continent. The region including all source-station Rayleigh wave paths (defined by geographical coordinates : -125,45 and 25,-75) was divided into cells of 2 by 2 degrees, and a group velocity for each cell (visited by at least one Rayleigh wave path) of the grid was computed. The estimated group velocities were then related to the Preliminary Reference Earth Model (PREM) and their percentual deviation from PREM were used to construct velocity maps at different periods (from 10 to 102 sec). The group velocity anomalies maps show a strong correlation with the superficial limits of the main geologic provinces in the region. Both Tocantis and Sao Francisco cratonic nuclei were clearly identified and they have deep roots. Several group velocity anomalies in the maps also have a direct correlation with recent studies about geoid anomalies in the southeastern Brazil and adjacent regions. The high density of Rayleigh wave paths across southeastern Brazil has provided high resolutions throughout the region under investigation. In general, the spatial resolution in the grid is of two degrees or 200km.

  19. Rayleigh-Taylor instability experiments in a cylindrically convergent geometry

    SciTech Connect

    Goodwin, B.; Weir, S.

    1995-08-25

    Due to the sensitivity of Rayleigh-Taylor instabilities to initial conditions and due to the difficulty of forming well controlled cylindrical or spherical fluid interfaces, Rayleigh-Taylor experiments are often performed with simple, planar interfaces. Rayleigh-Taylor instability phenomena of practical interest, however, (e.g., underwater explosions, supernova core collapses, and inertial confinement fusion capsule implosions) are typically associated with cylindrical or spherical interfaces in which convergent flow effects have an important influence on the dynamics of instability growth. Recently, Meshkov et.al. have developed a novel technique for studying Rayleigh-Taylor instability growth in a cylindrically convergent geometry. Their experiments utilized low-strength gelatin rings which are imploded by a detonating gas mixture of oxygen and acetylene. Since the gelatin itself has sufficient strength to resist significant deformation by gravity, no membranes are needed to define the ring shape. This experimental technique is attractive because it offers a high degree of control over the interfacial geometry and over the material`s strength and rigidity, which can be varied by adjusting the gelatin concentration. Finally, since both the gelatin and the explosive product gases are transparent, optical diagnostics can be used.

  20. Rayleigh Taylor instability of viscoelastic drops at high Weber numbers

    NASA Astrophysics Data System (ADS)

    Joseph, D. D.; Beavers, G. S.; Funada, T.

    2002-02-01

    Movies of the breakup of viscous and viscoelastic drops in the high-speed airstream behind a shock wave in a shock tube have been reported by Joseph, Belanger & Beavers (1999). They performed a Rayleigh Taylor stability analysis for the initial breakup of a drop of Newtonian liquid and found that the most unstable Rayleigh Taylor wave fits nearly perfectly with waves measured on enhanced images of drops from the movies, but the effects of viscosity cannot be neglected. Here we construct a Rayleigh Taylor stability analysis for an Oldroyd-B fluid using measured data for acceleration, density, viscosity and relaxation time [lambda]1. The most unstable wave is a sensitive function of the retardation time [lambda]2 which fits experiments when [lambda]2/[lambda]1 = O(10-3). The growth rates for the most unstable wave are much larger than for the comparable viscous drop, which agrees with the surprising fact that the breakup times for viscoelastic drops are shorter. We construct an approximate analysis of Rayleigh Taylor instability based on viscoelastic potential flow which gives rise to nearly the same dispersion relation as the unapproximated analysis.

  1. Modified Rayleigh distribution of wave heights in transitional water depths

    NASA Astrophysics Data System (ADS)

    Wang, Ying-guang

    2016-06-01

    This paper concerns the calculation of wave height exceedance probabilities for nonlinear irregular waves in transitional water depths, and a Transformed Rayleigh method is first proposed for carrying out the calculation. In the proposed Transformed Rayleigh method, the transformation model is chosen to be a monotonic exponential function, calibrated such that the first three moments of the transformed model match the moments of the true process. The proposed new method has been applied for calculating the wave height exceedance probabilities of a sea state with the surface elevation data measured at the Poseidon platform. It is demonstrated in this case that the proposed new method can offer better predictions than those by using the conventional Rayleigh wave height distribution model. The proposed new method has been further applied for calculating the total horizontal loads on a generic jacket, and its accuracy has once again been substantiated. The research findings gained from this study demonstrate that the proposed Transformed Rayleigh model can be utilized as a promising alternative to the well-established nonlinear wave height distribution models.

  2. Some observations of a sheared Rayleigh-Taylor/Benard instability

    NASA Technical Reports Server (NTRS)

    Humphrey, J. A. C.; Marcus, D. L.

    1987-01-01

    An account is provided of preliminary flow visualization observations made in an unstably stratified flow with shear superimposed. The structures observed appear to be the superposition of a Rayleigh-Taylor/Benard instability and a Kelvin-Helmholtz instability. Aside from its intrinsic fundamental value, the study of these structures is of special interest to theoreticians developing nonlinear stability calculation methodologies.

  3. Approximation for the Rayleigh Resolution of a Circular Aperture

    ERIC Educational Resources Information Center

    Mungan, Carl E.

    2009-01-01

    Rayleigh's criterion states that a pair of point sources are barely resolved by an optical instrument when the central maximum of the diffraction pattern due to one source coincides with the first minimum of the pattern of the other source. As derived in standard introductory physics textbooks, the first minimum for a rectangular slit of width "a"…

  4. Rayleigh, Ramsay, Rutherford and Raman--their connections with, and contributions to, the discovery of the Raman effect.

    PubMed

    Clark, Robin J H

    2013-02-21

    The key contributions of the four great Nobel Laureates - Lord Rayleigh, Sir William Ramsay, Lord Rutherford and Sir Chandrasekhara Raman - to the understanding of light scattering, to the identification and classification of the rare gases, and to the discovery in 1928 of the Raman effect are outlined. The interactions between these scientists are explored, in particular those of Rayleigh with Ramsay (in establishing the physics and chemistry of the rare gases), Ramsay with Rutherford (on studies of the radioactivity of radium dibromide and on the discovery of radon and its position in the periodic table), and Rutherford with Raman (in supporting Raman's career via the Royal Society and as a nominee for the Nobel Prize). The resilience and dedication of these scientific pioneers is emphasised, noting in particular that Rutherford and Raman emerged with success from unlikely backgrounds and from countries far removed from the then centres of scientific excellence. Key developments from 1928 onwards in the light sources used for the excitation of Raman spectra and in the detectors of Raman scattered radiation are outlined. Attention is drawn to the mounting number of scientific areas which continue to be opened up by Raman microscopy and many other derived techniques such as SERS, TERS, etc.

  5. Retrieval of Rayleigh Wave Ellipticity from Ambient Vibration Recordings

    NASA Astrophysics Data System (ADS)

    Maranò, Stefano; Hobiger, Manuel; Fäh, Donat

    2017-01-01

    The analysis of ambient vibrations is a useful tool in microzonation and geotechnical investigations. Ambient vibrations are composed to a large part of surface waves, both Love and Rayleigh waves. One reason to analyse surface waves is that they carry information about the subsurface. The dispersion curve of Rayleigh waves and Love waves can be retrieved using array processing techniques. The Rayleigh wave ellipticity, including the sense of rotation of the particle motion, can also be retrieved using array techniques. These quantities are used in an inversion procedure aimed at obtaining a structural model of the subsurface. The focus of this work is the retrieval of Rayleigh wave ellipticity. We show applications of the (ML) method presented in Maranó et al. (2012) to a number of sites in Switzerland. The sites examined are chosen to reflect a wide range of soil conditions that are of interest in microzonation studies. Using a synthetic wavefield with known structural model, we compare our results with theoretical ellipticity curves and we show the accuracy of the considered algorithm. The sense of rotation of the particle motion (prograde vs. retrograde) is also estimated. In addition, we show that by modelling the presence of both Love and Rayleigh waves it is possible to mitigate the disruptive influence of Love waves on the estimation of Rayleigh wave ellipticity. Using recordings from several real sites, we show that it is possible to retrieve the ellipticity curve over a broad range of frequencies. Fundamental modes and higher modes are retrieved. Singularities of the ellipticity, corresponding to a change of the sense of rotation from prograde to retrograde (or vice versa), are detected with great accuracy. Knowledge of Rayleigh wave ellipticity, including the sense of rotation, is useful in several ways. The ellipticity angle allows us to pinpoint accurately the frequency of singularities (i.e., peaks and zeros of the H/V representation of the

  6. Effect of molecular anisotropy on the intensity and degree of polarization of light scattered from model atmospheres

    NASA Technical Reports Server (NTRS)

    Bahethi, O. P.; Fraser, R. S.

    1975-01-01

    Computations of the intensity, flux, degree of polarization, and the positions of neutral points are presented for models of the terrestrial gaseous and hazy atmospheres by incorporating the molecular anisotropy due to air in the Rayleigh scattering optical thickness and phase matrix. Molecular anisotropy causes significant changes in the intensity, flux and the degree of polarization of the scattered light. The positions of neutral points do not change significantly. When the Rayleigh scattering optical thickness is kept constant and the molecular anisotropy factor is included only in the Rayleigh phase matrix, the flux does not change and the intensity and positions of neutron points change by a small amount. The changes in the degree of polarization are still significant.

  7. Scattering of light from metamaterial gratings with finite length.

    PubMed

    Grünhut, Vivian; Cuevas, Mauro; Depine, Ricardo A

    2012-06-01

    Using an integral equation approach based on the Rayleigh hypothesis, we investigate the scattering of a plane wave at the rough surface of a metamaterial with a finite number of sinusoidal grooves. To show the adequacy of the model, we present results that are in agreement with the predictions of physical optics and that quantitatively reproduce the polarization and angular dependences predicted by the C-formalism for metamaterial gratings with an infinite number of grooves.

  8. Passive Seismic Artillery Location by Exact Inverse Scattering,

    DTIC Science & Technology

    1980-07-01

    DOMAIN A VI NUMERICO -EXPERIMENTAL RESULTS 11 VII RECORIMENDATIONS FOR FUTURE RESEARCH 17 VIlI REFERENCES 19 IX APPENDIX: EXACT INVERSE SCATTERING THEORY...these numerico -experimental results, recomnendations for future research are made in section VII. A_ I I SECTION II REFORMULATION OF THE RAYLEIGH...N00014-76-C-0082) in the latter part of this research. This solution was numerico -experimentally verified for a point source and 11 I a point source

  9. Nonlinear light scattering in a carbon nanotube suspension

    SciTech Connect

    Mikheev, Gen M; Mogileva, T N; Bulatov, D L; Vanyukov, V V; Okotrub, Aleksandr V

    2010-01-31

    Nonlinear scattering of 1064-nm laser light in an aqueous suspension of purified carbon nanotubes has been studied in relation to their optical power limiting behaviour using z-scan measurements to simultaneously determine the energy and shape of the transmitted and 90{sup 0} circ-scattered pulses. The results indicate that the reduction in transmitted laser pulse energy with increasing incident power density is mainly due to the associated increase in scattered pulse energy. The shape, duration and time shift of the transmitted and 90{sup 0} circ-scattered pulses are intricate functions of incident power density. The data are interpreted in terms of thermally induced nonlinear and Rayleigh scattering processes at high and low incident power densities, respectively. (nonlinear optics phenomena)

  10. Q-space analysis of light scattering by ice crystals

    NASA Astrophysics Data System (ADS)

    Heinson, Yuli W.; Maughan, Justin B.; Ding, Jiachen; Chakrabarti, Amitabha; Yang, Ping; Sorensen, Christopher M.

    2016-12-01

    Q-space analysis is applied to extensive simulations of the single-scattering properties of ice crystals with various habits/shapes over a range of sizes. The analysis uncovers features common to all the shapes: a forward scattering regime with intensity quantitatively related to the Rayleigh scattering by the particle and the internal coupling parameter, followed by a Guinier regime dependent upon the particle size, a complex power law regime with incipient two dimensional diffraction effects, and, in some cases, an enhanced backscattering regime. The effects of significant absorption on the scattering profile are also studied. The overall features found for the ice crystals are similar to features in scattering from same sized spheres.

  11. Modeling of optical wireless scattering communication channels over broad spectra.

    PubMed

    Liu, Weihao; Zou, Difan; Xu, Zhengyuan

    2015-03-01

    The air molecules and suspended aerosols help to build non-line-of-sight (NLOS) optical scattering communication links using carriers from near infrared to visible light and ultraviolet bands. This paper proposes channel models over such broad spectra. Wavelength dependent Rayleigh and Mie scattering and absorption coefficients of particles are analytically obtained first. They are applied to the ray tracing based Monte Carlo method, which models the photon scattering angle from the scatterer and propagation distance between two consecutive scatterers. Communication link path loss is studied under different operation conditions, including visibility, particle density, wavelength, and communication range. It is observed that optimum communication performances exist across the wavelength under specific atmospheric conditions. Infrared, visible light and ultraviolet bands show their respective features as conditions vary.

  12. Dense Matter Characterization by X-ray Thomson Scattering

    SciTech Connect

    Landen, O L; Glenzer, S H; Edwards, M J; Lee, R W; Collins, G W; Cauble, R C; Hsing, W W; Hammel, B A

    2000-12-29

    We discuss the extension of the powerful technique of Thomson scattering to the x-ray regime for providing an independent measure of plasma parameters for dense plasmas. By spectrally-resolving the scattering, the coherent (Rayleigh) unshifted scattering component can be separated from the incoherent Thomson component, which is both Compton and Doppler shifted. The free electron density and temperature can then be inferred from the spectral shape of the high frequency Thomson scattering component. In addition, as the plasma temperature is decreased, the electron velocity distribution as measured by incoherent Thomson scattering will make a transition from the traditional Gaussian Boltzmann distribution to a density-dependent parabolic Fermi distribution to. We also present a discussion for a proof-of-principle experiment appropriate for a high energy laser facility.

  13. Scattering by Randomly Oriented Thin Ice Disks with Moderate Equivalent-Sphere Size Parameters

    NASA Technical Reports Server (NTRS)

    Zakharova, Nadia T.; Mishchenko, Michael I.; Hansen, James E. (Technical Monitor)

    2001-01-01

    We use the T-matrix method to compute the scattering matrix for randomly oriented circular ice cylinders with diameter-to-length ratios 1 and 20 and surface-equivalent-sphere size parameters up to 12. We show that wavelength-sized, sharp-edged ice plates with extreme diameter-to-length ratios possess the same scattering properties as smooth plate-like spheroids: their phase functions are similar to those of surface-equivalent compact particles, whereas all other elements of the scattering matrix are typical of Rayleigh scattering.

  14. Angle-Resolved Second-Harmonic Light Scattering from Colloidal Particles

    SciTech Connect

    Yang, N.; Angerer, W. E.; Yodh, A. G.

    2001-09-03

    We report angle-resolved second-harmonic generation (SHG) measurements from suspensions of centrosymmetric micron-size polystyrene spheres with surface-adsorbed dye (malachite green). The second-harmonic scattering profiles differ qualitatively from linear light scattering profiles of the same particles. We investigated these radiation patterns using several polarization configurations and particle diameters. We introduce a simple Rayleigh-Gans-Debye model to account for the SHG scattering anisotropy. The model compares favorably with our experimental data. Our measurements suggest scattering anisotropy may be used to isolate particle nonlinear optics from other bulk nonlinear optical effects in suspension.

  15. Ultraviolet Rayleigh-Mie lidar by use of a multicavity Fabry-Perot filter for accurate temperature profiling of the troposphere.

    PubMed

    Hua, Dengxin; Kobayashi, Takao

    2005-10-20

    A UV Rayleigh-Mie scattering lidar system at 355 nm has been upgraded for more-accurate temperature profiling of the troposphere by use of a new multicavity Fabry-Perot etalon (MCFPE) filter. The MCFPE filter, which was designed to improve the stability and operational characteristics of the lidar system, has three filter bandpass functions and separates one Mie scattering and two Rayleigh scattering signals from the lidar return signal and simultaneously acts as a laser frequency discriminator to lock the laser frequency. Moreover, a high-resolution grating is employed to block signal interference from Raman scattering and the solar background. A practical lidar system, which features strong system stabilization and high measurement accuracy, has been built, and the performance of the lidar system has been verified by comparison of temperature profiling between the lidar and a radiosonde. Good agreement between the two instrument measurements was obtained in terms of lapse rate and inversion layer height. Statistical temperature errors of less than 1 K up to a height of 3 km are obtainable with 5 min observation time for daytime measurements.

  16. Characterization of Non-Rayleigh Acoustic Scattering by Elongated Scatterers in the Water Column and on Boundaries

    DTIC Science & Technology

    2013-01-30

    key results in the literature (#1) and advancing the field (#2 and #3): aoV^oWHI 1. Key results of Ehrenberg (1972) involving the echo statistics of... Ehrenberg (1972) "A method for extracting the fish target strength distribution from acoustic echoes," in Proc. Conf. Eng. Ocean Environ., Vol. 1

  17. Optical scattering lengths in large liquid-scintillator neutrino detectors

    SciTech Connect

    Wurm, M.; Feilitzsch, F. von; Goeger-Neff, M.; Hofmann, M.; Lewke, T.; Meindl, Q.; Moellenberg, R.; Oberauer, L.; Potzel, W.; Tippmann, M.; Todor, S.; Winter, J.; Lachenmaier, T.; Traunsteiner, C.; Undagoitia, T. Marrodan

    2010-05-15

    For liquid-scintillator neutrino detectors of kiloton scale, the transparency of the organic solvent is of central importance. The present paper reports on laboratory measurements of the optical scattering lengths of the organic solvents phenylxylylethane, linear alkylbenzene (LAB), and dodecane, which are under discussion for next-generation experiments such as SNO+ (Sudbury Neutrino Observatory), HanoHano, or LENA (Low Energy Neutrino Astronomy). Results comprise the wavelength range of 415-440 nm. The contributions from Rayleigh and Mie scattering as well as from absorption/re-emission processes are discussed. Based on the present results, LAB seems to be the preferred solvent for a large-volume detector.

  18. Optical scattering lengths in large liquid-scintillator neutrino detectors.

    PubMed

    Wurm, M; von Feilitzsch, F; Göger-Neff, M; Hofmann, M; Lachenmaier, T; Lewke, T; Marrodán Undagoitia, T; Meindl, Q; Möllenberg, R; Oberauer, L; Potzel, W; Tippmann, M; Todor, S; Traunsteiner, C; Winter, J

    2010-05-01

    For liquid-scintillator neutrino detectors of kiloton scale, the transparency of the organic solvent is of central importance. The present paper reports on laboratory measurements of the optical scattering lengths of the organic solvents phenylxylylethane, linear alkylbenzene (LAB), and dodecane, which are under discussion for next-generation experiments such as SNO+ (Sudbury Neutrino Observatory), HanoHano, or LENA (Low Energy Neutrino Astronomy). Results comprise the wavelength range of 415-440 nm. The contributions from Rayleigh and Mie scattering as well as from absorption/re-emission processes are discussed. Based on the present results, LAB seems to be the preferred solvent for a large-volume detector.

  19. Hyperfine Coherence in the Presence of Spontaneous Photon Scattering

    NASA Astrophysics Data System (ADS)

    Ozeri, R.; Langer, C.; Jost, J. D.; Demarco, B.; Ben-Kish, A.; Blakestad, B. R.; Britton, J.; Chiaverini, J.; Itano, W. M.; Hume, D. B.; Leibfried, D.; Rosenband, T.; Schmidt, P. O.; Wineland, D. J.

    2005-07-01

    The coherence of a hyperfine-state superposition of a trapped 9Be+ ion in the presence of off-resonant light is studied experimentally. It is shown that Rayleigh elastic scattering of photons that does not change state populations also does not affect coherence. We observe coherence times that exceed the average scattering time of 19 photons which is determined from measured Stark shifts. This result implies that, with sufficient control over its parameters, laser light can be used to manipulate hyperfine-state superpositions with very little decoherence.

  20. Cloaking of solar cell contacts at the onset of Rayleigh scattering

    PubMed Central

    San Román, Etor; Vitrey, Alan; Buencuerpo, Jerónimo; Prieto, Iván; Llorens, José M.; García-Martín, Antonio; Alén, Benito; Chaudhuri, Anabil; Neumann, Alexander; Brueck, S. R. J.; Ripalda, José M.

    2016-01-01

    Electrical contacts on the top surface of solar cells and light emitting diodes cause shadow losses. The phenomenon of extraordinary optical transmission through arrays of subwavelength holes suggests the possibility of engineering such contacts to reduce the shadow using plasmonics, but resonance effects occur only at specific wavelengths. Here we describe instead a broadband effect of enhanced light transmission through arrays of subwavelength metallic wires, due to the fact that, in the absence of resonances, metal wires asymptotically tend to invisibility in the small size limit regardless of the fraction of the device area taken up by the contacts. The effect occurs for wires more than an order of magnitude thicker than the transparency limit for metal thin films. Finite difference in time domain calculations predict that it is possible to have high cloaking efficiencies in a broadband wavelength range, and we experimentally demonstrate contact shadow losses less than half of the geometric shadow. PMID:27339390

  1. Coherent Rayleigh-Brillouin Scattering in High Intensity Laser Fields: Optical Lattice gas Heating (Briefing Charts)

    DTIC Science & Technology

    2012-07-01

    ADDRESS(ES) 8. PERFORMING ORGANIZATION REPORT NO. Air Force Research Laboratory (AFMC) AFRL/RQRC 10 E. Saturn Blvd. Edwards AFB CA 93524-7680...unlimited CRBS Results Low Intensity • Experiment and DSMC show good agreement with six-moment model (s6) for low intensity (X. Pan , “Coherent

  2. Cloaking of solar cell contacts at the onset of Rayleigh scattering.

    PubMed

    San Román, Etor; Vitrey, Alan; Buencuerpo, Jerónimo; Prieto, Iván; Llorens, José M; García-Martín, Antonio; Alén, Benito; Chaudhuri, Anabil; Neumann, Alexander; Brueck, S R J; Ripalda, José M

    2016-06-24

    Electrical contacts on the top surface of solar cells and light emitting diodes cause shadow losses. The phenomenon of extraordinary optical transmission through arrays of subwavelength holes suggests the possibility of engineering such contacts to reduce the shadow using plasmonics, but resonance effects occur only at specific wavelengths. Here we describe instead a broadband effect of enhanced light transmission through arrays of subwavelength metallic wires, due to the fact that, in the absence of resonances, metal wires asymptotically tend to invisibility in the small size limit regardless of the fraction of the device area taken up by the contacts. The effect occurs for wires more than an order of magnitude thicker than the transparency limit for metal thin films. Finite difference in time domain calculations predict that it is possible to have high cloaking efficiencies in a broadband wavelength range, and we experimentally demonstrate contact shadow losses less than half of the geometric shadow.

  3. Cloaking of solar cell contacts at the onset of Rayleigh scattering

    NASA Astrophysics Data System (ADS)

    San Román, Etor; Vitrey, Alan; Buencuerpo, Jerónimo; Prieto, Iván; Llorens, José M.; García-Martín, Antonio; Alén, Benito; Chaudhuri, Anabil; Neumann, Alexander; Brueck, S. R. J.; Ripalda, José M.

    2016-06-01

    Electrical contacts on the top surface of solar cells and light emitting diodes cause shadow losses. The phenomenon of extraordinary optical transmission through arrays of subwavelength holes suggests the possibility of engineering such contacts to reduce the shadow using plasmonics, but resonance effects occur only at specific wavelengths. Here we describe instead a broadband effect of enhanced light transmission through arrays of subwavelength metallic wires, due to the fact that, in the absence of resonances, metal wires asymptotically tend to invisibility in the small size limit regardless of the fraction of the device area taken up by the contacts. The effect occurs for wires more than an order of magnitude thicker than the transparency limit for metal thin films. Finite difference in time domain calculations predict that it is possible to have high cloaking efficiencies in a broadband wavelength range, and we experimentally demonstrate contact shadow losses less than half of the geometric shadow.

  4. Characterizing a Co-Flow Nozzle for use in a Filtered Rayleigh Scattering System

    DTIC Science & Technology

    2006-06-01

    Figure 16- Gridgen model imported from Solid Works ................................................... 42 Figure 17-Cutaway Gridgen model showing...selected domains ....................................... 45 Figure 18- Gridgen model showing the three axis cell distribution of the Gridgen model...Close in picture of the cell distribution of the Gridgen model around a support vane

  5. Development of Terahertz Rayleigh Scattering Diagnostics for a Solid Rocket Exhaust Plume

    DTIC Science & Technology

    2010-10-28

    Approved for public release. Distribution unlimited. The views expressed in this article are those of the author and do not...the atmospheric properties of other large bodies such as asteroids and comets. These characteristics can lead to improvements in the models of

  6. Tunable Wavelength Solid-State Lasers and Turbulent Jet Diagnostics by Rayleigh and Fluorescence Scattering.

    DTIC Science & Technology

    1981-09-01

    We did not succeed in achieving laser action from Eu 2+ ions doped in CaF 2, BaF2, SrF2 , CaCl 2, BaC1 2, SrCl2, BaCIF, and SrCIF crystals even...laser action from Ce ions doped in CaF2, BaF2, SrF2 , and LaF3 (see Appendix B). Two other research groups also reported their failures to 3+ achieve laser...sequently, the fact that laser emission for Ce3+ ions is achievable in YLF, and not in YAG, CaF2, BaF2, SrF2 , and LaF3, clearly demonstrates that even a

  7. Measurement of spin coherence using Raman scattering

    NASA Astrophysics Data System (ADS)

    Sun, Z.; Delteil, A.; Faelt, S.; Imamoǧlu, A.

    2016-06-01

    Ramsey interferometry provides a natural way to determine the coherence time of most qubit systems. Recent experiments on quantum dots, however, demonstrated that dynamical nuclear spin polarization can strongly influence the measurement process, making it difficult to extract the T2* coherence time using standard optical Ramsey pulses. Here, we demonstrate an alternative method for spin coherence measurement that is based on first-order coherence of photons generated in spin-flip Raman scattering. We show that if a quantum emitter is driven by a weak monochromatic laser, Raman coherence is determined exclusively by spin coherence, allowing for a direct determination of spin T2* time. When combined with coherence measurements on Rayleigh scattered photons, our technique enables us to identify coherent and incoherent contributions to resonance fluorescence, and to minimize the latter. We verify the validity of our technique by comparing our results to those determined from Ramsey interferometry for electron and heavy-hole spins.

  8. Sustained shear flows in Rayleigh-Bénard convection

    NASA Astrophysics Data System (ADS)

    Quist, Tayler; Anders, Evan; Brown, Benjamin; Oishi, Jeffrey

    2016-11-01

    Zonal shear flows play important roles in both the solar and geo dynamos. In two dimensional simulations, and at relatively narrow aspect ratios, Rayleigh-Bénard convection naturally achieves zonal shear flows. These zonal flows are driven by the convection and modify it, significantly altering the heat transport and convective structures. Here we study shear flows in two and three-dimensional simulations of Rayleigh-Bénard convection using the Dedalus pseudospectral framework. At small aspect ratios and at Prandtl number 1, a large horizontal shear naturally occurs. At larger aspect ratios, we find that shearing is naturally prevented unless manually induced; there is a bistability between states dominated by "flywheel" modes and states dominated by large scale shear. We explore these states and the possibilities of sustained large scale shear in 3-D simulations.

  9. Fatigue Crack Growth Monitoring Using Rayleigh-Like Waves

    NASA Astrophysics Data System (ADS)

    Masserey, B.; Fromme, P.

    2010-02-01

    A common problem in aircraft maintenance is the development of fatigue cracks at fasteners due to stress concentration. The use of Rayleigh-like waves for the monitoring of fatigue crack growth at a fastener hole in tensile, aluminum specimens is investigated. Rayleigh-like waves can propagate along the structure and have good sensitivity for the detection of small defects. They are excited in the specimen during fatigue experiments using standard wedge transducers and measured using laser interferometry. Fatigue crack growth during cyclic loading is monitored optically and the changes in the ultrasonic signal caused by crack growth are quantified. The laser measurements show a good sensitivity for the early detection of fatigue damage.

  10. Is the magnetopause Rayleigh-Taylor unstable sometimes?

    SciTech Connect

    Gratton, F.T.; Farrugia, C.J.; Cowley, S.W.H.

    1996-03-01

    The authors examine the question of whether the magnetopause is Rayleigh-Taylor stable. The magnetopause tends to be in continuous motion because of the effect of the dyanmic pressure from the solar wind. When there is a sudden drop in solar wind pressure, and the magnetopause tends to accelerate sunward, a situation is created where the magnetopause may go unstable. The authors look at two possible stabilizing effects, first the magnetic shear which exists across the magnetopause, and then the viscous nature of the magnetosheath plasma. They find that large shear leads to stability for the Rayleigh-Taylor mode. When there is a strong northward component in the magnetosheath field, they find that the magnetopause may be unstable to this mode for both global and internal modes. They also discuss the effect of such instabilities on observations.

  11. Joint inversion of fundamental and higher mode Rayleigh waves

    USGS Publications Warehouse

    Luo, Y.-H.; Xia, J.-H.; Liu, J.-P.; Liu, Q.-S.

    2008-01-01

    In this paper, we analyze the characteristics of the phase velocity of fundamental and higher mode Rayleigh waves in a six-layer earth model. The results show that fundamental mode is more sensitive to the shear velocities of shallow layers (< 7 m) and concentrated in a very narrow band (around 18 Hz) while higher modes are more sensitive to the parameters of relatively deeper layers and distributed over a wider frequency band. These properties provide a foundation of using a multi-mode joint inversion to define S-wave velocity. Inversion results of both synthetic data and a real-world example demonstrate that joint inversion with the damped least squares method and the SVD (Singular Value Decomposition) technique to invert Rayleigh waves of fundamental and higher modes can effectively reduce the ambiguity and improve the accuracy of inverted S-wave velocities.

  12. Nonlinear mixing of laser generated narrowband Rayleigh surface waves

    NASA Astrophysics Data System (ADS)

    Bakre, Chaitanya; Rajagopal, Prabhu; Balasubramaniam, Krishnan

    2017-02-01

    This research presents the nonlinear mixing technique of two co-directionally travelling Rayleigh surface waves generated and detected using laser ultrasonics. The optical generation of Rayleigh waves on the specimen is obtained by shadow mask method. In conventional nonlinear measurements, the inherently small higher harmonics are greatly influenced by the nonlinearities caused by coupling variabilities and surface roughness between the transducer and specimen interface. The proposed technique is completely contactless and it should be possible to eliminate this problem. Moreover, the nonlinear mixing phenomenon yields not only the second harmonics, but also the sum and difference frequency components, which can be used to measure the acoustic nonlinearity of the specimen. In this paper, we will be addressing the experimental configurations for this technique. The proposed technique is validated experimentally on Aluminum 7075 alloy specimen.

  13. Singularities in water waves and Rayleigh-Taylor instability

    NASA Technical Reports Server (NTRS)

    Tanveer, S.

    1991-01-01

    Singularities in inviscid two-dimensional finite-amplitude water waves and inviscid Rayleigh-Taylor instability are discussed. For the deep water gravity waves of permanent form, through a combination of analytical and numerical methods, results describing the precise form, number, and location of singularities in the unphysical domain as the wave height is increased are presented. It is shown how the information on the singularity in the unphysical region has the same form as for deep water waves. However, associated with such a singularity is a series of image singularities at increasing distances from the physical plane with possibly different behavior. Furthermore, for the Rayleigh-Taylor problem of motion of fluid over a vacuum and for the unsteady water wave problem, integro-differential equations valid in the unphysical region are derived, and how these equations can give information on the nature of singularities for arbitrary initial conditions is shown.

  14. Analysis of Rayleigh wave interactions for surface crack characterization

    NASA Astrophysics Data System (ADS)

    Rosli, M. H.; Fan, Y.; Edwards, R. S.

    2012-05-01

    Electromagnetic acoustic transducers (EMATs) have been used in pitch-catch mode for a better characterization of surface cracks in metals. The system, which combines the measurement of Rayleigh wave velocity in the in-plane and out-of-plane directions, has been used to understand the interaction of Rayleigh waves with inclined surface cracks. This shows a stronger and more prominent enhancement pattern when compared to the enhancement caused by cracks which are normal to the surface. In addition, measurements in the far-field are combined with the near-field enhancement measurement, with a view to characterize the cracks. An algorithm for characterizing surface cracks is presented. A finite element method model has been computed to simulate the experiment, and the cause of the prominent enhancement in the inclined cracks is explained.

  15. Measurement of magnetic field using Rayleigh backscattering in optical fibres

    SciTech Connect

    Wuilpart, M.; Caucheteur, C.; Goussarov, A.; Aerssens, M.; Massaut, V.; Megret, P.

    2011-07-01

    In this paper, we investigate the use of optical reflectometry in optical fibres for the measurement of magnetic field. The dedicated application concerns the measurement of plasma current in the fusion reactor. The measurement is based on the rotation of the polarization state of the Rayleigh backscattered signal when an optical pulse is launched in the fibre. Particular care has been undertaken to evaluate the impact of linear birefringence on the measurement performance. (authors)

  16. Dipping-interface mapping using mode-separated Rayleigh waves

    USGS Publications Warehouse

    Luo, Y.; Xia, J.; Xu, Y.; Zeng, C.; Miller, R.D.; Liu, Q.

    2009-01-01

    Multichannel analysis of surface waves (MASW) method is a non-invasive geophysical technique that uses the dispersive characteristic of Rayleigh waves to estimate a vertical shear (S)-wave velocity profile. A pseudo-2D S-wave velocity section is constructed by aligning 1D S-wave velocity profiles at the midpoint of each receiver spread that are contoured using a spatial interpolation scheme. The horizontal resolution of the section is therefore most influenced by the receiver spread length and the source interval. Based on the assumption that a dipping-layer model can be regarded as stepped flat layers, high-resolution linear Radon transform (LRT) has been proposed to image Rayleigh-wave dispersive energy and separate modes of Rayleigh waves from a multichannel record. With the mode-separation technique, therefore, a dispersion curve that possesses satisfactory accuracy can be calculated using a pair of consecutive traces within a mode-separated shot gather. In this study, using synthetic models containing a dipping layer with a slope of 5, 10, 15, 20, or 30 degrees and a real-world example, we assess the ability of using high-resolution LRT to image and separate fundamental-mode Rayleigh waves from raw surface-wave data and accuracy of dispersion curves generated by a pair of consecutive traces within a mode-separated shot gather. Results of synthetic and real-world examples demonstrate that a dipping interface with a slope smaller than 15 degrees can be successfully mapped by separated fundamental waves using high-resolution LRT. ?? Birkh??user Verlag, Basel 2009.

  17. Rayleigh-Taylor instability in an equal mass plasma

    SciTech Connect

    Adak, Ashish; Ghosh, Samiran; Chakrabarti, Nikhil

    2014-09-15

    The Rayleigh-Taylor (RT) instability in an inhomogeneous pair-ion plasma has been analyzed. Considering two fluid model for two species of ions (positive and negative), we obtain the possibility of the existence of RT instability. The growth rate of the RT instability as usual depends on gravity and density gradient scale length. The results are discussed in context of pair-ion plasma experiments.

  18. Rayleigh-Taylor vortices in a pair-ion plasma

    SciTech Connect

    Adak, Ashish Khan, Manoranjan

    2015-04-15

    The Rayleigh-Taylor (RT) vortices and the analytical solution of three-mode coupling in pair-ion plasmas are investigated. It is shown that the E×B convection of polarization drift is responsible for the saturation of growing RT instability and as a result the localized dipole vortex structures are formed. The shear flow generation due to the destruction of vortex structures is discussed by the Fourier mode analysis.

  19. Multimode Rayleigh wave profiling by hybrid surface and borehole methods

    NASA Astrophysics Data System (ADS)

    Lin, Shibin; Ashlock, Jeramy C.

    2014-05-01

    To improve the accuracy of shallow seismic shear wave velocity profiling, we propose a minimally invasive hybrid surface-and-borehole method that enhances the detection of higher modes of Rayleigh wave dispersion data. The new method combines techniques from the multichannel analysis of surface waves and multichannel simulation with one receiver (MSOR) methods to record components of Rayleigh wave motion at the surface as well as at shallow depths within the soil mass. The performance of the proposed method is demonstrated through computational and experimental studies. We show that individual modes of Rayleigh waves can exhibit different dominant depths at which their motion is most significant. This is demonstrated through a numerical study of eigenvectors of layered soil profiles via the stiffness matrix method, and confirmed by a finite element simulation of the apparent dispersion trends recorded at shallow depths using MSOR. Upon superimposing dispersion data recorded via the receivers at various depths, the resulting multimode dispersion data is used in a multi-objective inverse analysis, for which the difference between experimental and theoretical dispersive phase-velocity spectra are minimized for multiple modes simultaneously. In the numerical study, we demonstrate that the resulting inverted profiles and theoretical dispersion data have improved accuracy relative to single-mode inversion. Preliminary field tests are performed using the new hybrid method, and the results are shown to support the conclusions of the numerical study and confirm the feasibility of the proposed technique. Although the use of multiple modes in surface wave testing is not new, the proposed hybrid method can provide more accurate and complete multimodal dispersion data than achieved with surface-only Rayleigh wave methods. As a result, errors because of misidentification or partial measurement of higher modes may be minimized, thus reducing statistical uncertainty in the

  20. Rayleigh-Taylor instability in dusty plasma experiment

    SciTech Connect

    Avinash, K.; Sen, A.

    2015-08-15

    The stability of a stratified dust cloud levitated in an anodic plasma is studied in the weakly and strongly coupled dust regimes. It is shown that the cloud is predominantly unstable to a Rayleigh-Taylor (RT) instability driven by a component of the ambient gravity in a direction opposite to the direction of dust density stratification in the cloud. The elasticity of the strongly coupled dust is shown to set a threshold for the RT instability, which is consistent with experimental observations.

  1. Sensitivity of high-frequency Rayleigh-wave data revisited

    USGS Publications Warehouse

    Xia, J.; Miller, R.D.; Ivanov, J.

    2007-01-01

    Rayleigh-wave phase velocity of a layered earth model is a function of frequency and four groups of earth properties: P-wave velocity, S-wave velocity (Vs), density, and thickness of layers. Analysis of the Jacobian matrix (or the difference method) provides a measure of dispersion curve sensitivity to earth properties. Vs is the dominant influence for the fundamental mode (Xia et al., 1999) and higher modes (Xia et al., 2003) of dispersion curves in a high frequency range (>2 Hz) followed by layer thickness. These characteristics are the foundation of determining S-wave velocities by inversion of Rayleigh-wave data. More applications of surface-wave techniques show an anomalous velocity layer such as a high-velocity layer (HVL) or a low-velocity layer (LVL) commonly exists in near-surface materials. Spatial location (depth) of an anomalous layer is usually the most important information that surface-wave techniques are asked to provide. Understanding and correctly defining the sensitivity of high-frequency Rayleigh-wave data due to depth of an anomalous velocity layer are crucial in applying surface-wave techniques to obtain a Vs profile and/or determine the depth of an anomalous layer. Because depth is not a direct earth property of a layered model, changes in depth will result in changes in other properties. Modeling results show that sensitivity at a given depth calculated by the difference method is dependent on the Vs difference (contrast) between an anomalous layer and surrounding layers. The larger the contrast is, the higher the sensitivity due to depth of the layer. Therefore, the Vs contrast is a dominant contributor to sensitivity of Rayleigh-wave data due to depth of an anomalous layer. Modeling results also suggest that the most sensitive depth for an HVL is at about the middle of the depth to the half-space, but for an LVL it is near the ground surface. ?? 2007 Society of Exploration Geophysicists.

  2. Viscous Rayleigh-Taylor instability in spherical geometry

    DOE PAGES

    Mikaelian, Karnig O.

    2016-02-08

    We consider viscous fluids in spherical geometry, a lighter fluid supporting a heavier one. Chandrasekhar [Q. J. Mech. Appl. Math. 8, 1 (1955)] analyzed this unstable configuration providing the equations needed to find, numerically, the exact growth rates for the ensuing Rayleigh-Taylor instability. He also derived an analytic but approximate solution. We point out a weakness in his approximate dispersion relation (DR) and offer one that is to some extent improved.

  3. Seismic Response to Sonic Boom-Coupled Rayleigh Waves

    DTIC Science & Technology

    1990-06-28

    Alluvium Dalby Series (clay, very firm clay, silty clay; calcareous) Friends Series (fine sandy loam, friable loam, clay; slightly acid, noncalcareous...friable clay loam; calcareous) Vethalen clay (Ve) (clay, very firm clay, friable clay loam; calcareous) Verhalen- Dalby association (Vm) (50% to 80...Prospecting: 3rd edition. McGraw-Hill, New York. NY. 220 pp. Dobrin, M. B., R. F. Simon , & P. L. Lawrence, 1951, Rayleigh waves from small explosions

  4. Distribution and moments of radial error. [Rayleigh distribution - random variables

    NASA Technical Reports Server (NTRS)

    White, R. G.

    1975-01-01

    An investigation of the moments and probability distribution of the resultant of two normally distributed random variables is presented. This is the so-called generalized Rayleigh distribution which has many applications in the study of wind shear, random noise, and radar. The most general formula was derived, and two special cases were considered for which tables of the moments and probability distribution functions are included as an appendix. One of the special cases was generalized to n-dimensions.

  5. A Theoretical Light Scattering Model of Nanoparticle Laser Tweezers

    NASA Technical Reports Server (NTRS)

    Lock, James A.

    2003-01-01

    Accomplishments this reporting period include: 1. derived, programmed, checked, and tested the Mie light scattering theory formulas for the radiation trapping force for both the on-axis and off-axis geometry of the trapping beam plus trapped spherical particle; 2. verified that the computed radiation trapping force for a freely propagating focused Gaussian laser beam incident on a spherical particle agrees with previous published calculations; 3. compared the small particle size and large particle size limits of the Mie calculation with the results of Rayleigh scattering theory and ray scattering theory, respectively and verified that the comparison is correct for Rayleigh scattering theory but found that ray theory omits an important light scattering effect included in the Mie theory treatment; 4. generalized the calculation of the radiation trapping force on a spherical particle in the on-axis geometry from a freely propagating focused Gaussian laser beam to the realistic situation of a Gaussian beam truncated and focused by a high numerical aperture oil-immersion microscope objective lens and aberrated by the interface between the microscope cover slip and the liquid-filled sample volume; and 5. compared the calculated radiation trapping force for this geometry with the results of previously published experiments and found that the agreement is better than when using previously developed theories.

  6. Insight from a careful dissection of the Rayleigh Distillation Model

    NASA Astrophysics Data System (ADS)

    Vachon, R. W.; Welker, J. M.

    2010-12-01

    Generally, precipitation isotopes (δ18O and δD) become progressively depleted with colder temperatures of condensation. However the complexity and interactions between environmental factors provides considerable uncertainty in predicting the spatial and temporal isotopic patterns of precipitation. Models that include isotope components are often used for interpretations or reproductions of spatial and temporal isotope trends. In fact, the most basic yet widely used model, Rayleigh Distillation Model, takes into account a few fundamental climatological factors to describe global isotope patterns. This paper provides a fresh examination of the Rayleigh Model, which has a long history of applications to precipitation isotope analysis. Additionally, we quantify how changes in environmental parameters affect the way that precipitation isotopes relate to temperatures of equilibrium - a relationship that is often thought to faithfully reflect temperatures of condensation (particularly at the high latitudes). Temperature of condensation remains the most important variable to consider when using the Rayleigh Model to unravel seasonal isotopic trends. However, the degree that (i) the amplitude of seasonally oscillating moisture source temperatures, (ii) average annual temperature difference between source and terrestrial sink, and (iii) agreement of source phasing and terrestrial sink temperatures can significantly impact precipitation isotope concentration throughout a given year, thus the way that precipitation isotopes relate to temperatures of condensation.

  7. Anomalous shape of magnetic loops in the Rayleigh region

    NASA Astrophysics Data System (ADS)

    Seeck, St.; Lambeck, M.

    1995-11-01

    According to its congruency property, the Preisach model demands an equivalent shape of magnetic minor loops, the so-called Rayleigh loops. We measured these loops with an inductive setup and noticed a different anomalous shape of Rayleigh loops which depends on the magnetic history. Special materials (particularly recording media) show a concave-convex shape in contrast to the normal biconvex shape. This anomalous shape can be explained by combining the Preisach model with the Stoner-Wohlfarth model. It follows from this explanation that the degree of the anomaly depends on the material, especially in how far it fulfills the conditions of the Stoner-Wohlfarth model. The experiments show the effect that is expected according to the material. In this way the measurement of the anomalous Rayleigh loops can be used as a new method to test the Stoner-Wohlfarth properties of a material. This is more effective than using the Henkel plot [G. Bertotti and V. Basso, J. Appl. Phys. 73, 5827 (1993)].

  8. Model studies of Rayleigh instabilities via microdesigned interfaces

    SciTech Connect

    Glaeser, Andreas M.

    2000-10-17

    The energetic and kinetic properties of surfaces play a critical role in defining the microstructural changes that occur during sintering and high-temperature use of ceramics. Characterization of surface diffusion in ceramics is particularly difficult, and significant variations in reported values of surface diffusivities arise even in well-studied systems. Effects of impurities, surface energy anisotropy, and the onset of surface attachment limited kinetics (SALK) are believed to contribute to this variability. An overview of the use of Rayleigh instabilities as a means of characterizing surface diffusivities is presented. The development of models of morphological evolution that account for effects of surface energy anisotropy is reviewed, and the potential interplay between impurities and surface energy anisotropy is addressed. The status of experimental studies of Rayleigh instabilities in sapphire utilizing lithographically introduced pore channels of controlled geometry and crystallography is summarized. Results of model studies indicate that impurities can significantly influence both the spatial and temporal characteristics of Rayleigh instabilities; this is attributed at least in part to impurity effects on the surface energy anisotropy. Related model experiments indicate that the onset of SALK may also contribute significantly to apparent variations in surface diffusion coefficients.

  9. Turbulent Boundary Layer in High Rayleigh Number Convection in Air

    NASA Astrophysics Data System (ADS)

    du Puits, Ronald; Li, Ling; Resagk, Christian; Thess, André; Willert, Christian

    2014-03-01

    Flow visualizations and particle image velocimetry measurements in the boundary layer of a Rayleigh-Bénard experiment are presented for the Rayleigh number Ra =1.4×1010. Our visualizations indicate that the appearance of the flow structures is similar to ordinary (isothermal) turbulent boundary layers. Our particle image velocimetry measurements show that vorticity with both positive and negative sign is generated and that the smallest flow structures are 1 order of magnitude smaller than the boundary layer thickness. Additional local measurements using laser Doppler velocimetry yield turbulence intensities up to I=0.4 as in turbulent atmospheric boundary layers. From our observations, we conclude that the convective boundary layer becomes turbulent locally and temporarily although its Reynolds number Re ≈200 is considerably smaller than the value 420 underlying existing phenomenological theories. We think that, in turbulent Rayleigh-Bénard convection, the transition of the boundary layer towards turbulence depends on subtle details of the flow field and is therefore not universal.

  10. Leakage predictions for Rayleigh-step, helium-purge seals

    NASA Technical Reports Server (NTRS)

    Proctor, Margaret P.

    1988-01-01

    Rayleigh-step, helium purge, annular shaft seals, studied for use in liquid oxygen turbopumps, generate a hydrodynamic force that enables the seal to follow shaft perturbations. Hence, smaller clearances can be used to reduce seal leakage. FLOWCAL, a computer code developed by Mechanical Technology Incorporated, predicts gas flow rate through an annular seal with an axial pressure gradient. Analysis of a 50-mm Rayleigh-step, helium-purge, annular seal showed the flow rate increased axial pressure gradient, downstream pressure, and eccentricity ratio. Increased inlet temperature reduced leakage. Predictions made at maximum and minimum clearances (due to centrifugal and thermal growths, machining tolerances and + or - 2 percent uncertainty in the clearance measurement) placed wide boundaries on expected flow rates. The widest boundaries were set by thermal growth conditions. Predicted flow rates for a 50-mm Rayleigh-step, helium-purge, annular seal underestimated measured flow rates by three to seven times. However, the analysis did accurately predict flow rates for choked gas flow through annular seals when compared to flow rates measured in two other independent studies.

  11. The upgrade of the Thomson scattering system for measurement on the C-2/C-2U devices

    NASA Astrophysics Data System (ADS)

    Zhai, K.; Schindler, T.; Kinley, J.; Deng, B.; Thompson, M. C.

    2016-11-01

    The C-2/C-2U Thomson scattering system has been substantially upgraded during the latter phase of C-2/C-2U program. A Rayleigh channel has been added to each of the three polychromators of the C-2/C-2U Thomson scattering system. Onsite spectral calibration has been applied to avoid the issue of different channel responses at different spots on the photomultiplier tube surface. With the added Rayleigh channel, the absolute intensity response of the system is calibrated with Rayleigh scattering in argon gas from 0.1 to 4 Torr, where the Rayleigh scattering signal is comparable to the Thomson scattering signal at electron densities from 1 × 1013 to 4 × 1014 cm-3. A new signal processing algorithm, using a maximum likelihood method and including detailed analysis of different noise contributions within the system, has been developed to obtain electron temperature and density profiles. The system setup, spectral and intensity calibration procedure and its outcome, data analysis, and the results of electron temperature/density profile measurements will be presented.

  12. Nonlinear Laplacian spectral analysis of Rayleigh-Bénard convection

    NASA Astrophysics Data System (ADS)

    Brenowitz, N. D.; Giannakis, D.; Majda, A. J.

    2016-06-01

    The analysis of physical datasets using modern methods developed in machine learning presents unique challenges and opportunities. These datasets typically feature many degrees of freedom, which tends to increase the computational cost of statistical methods and complicate interpretation. In addition, physical systems frequently exhibit a high degree of symmetry that should be exploited by any data analysis technique. The classic problem of Rayleigh Benárd convection in a periodic domain is an example of such a physical system with trivial symmetries. This article presents a technique for analyzing the time variability of numerical simulations of two-dimensional Rayleigh-Bénard convection at large aspect ratio and intermediate Rayleigh number. The simulated dynamics are highly unsteady and consist of several convective rolls that are distributed across the domain and oscillate with a preferred frequency. Intermittent extreme events in the net heat transfer, as quantified by the time-weighted probability distribution function of the Nusselt number, are a hallmark of these simulations. Nonlinear Laplacian Spectral Analysis (NLSA) is a data-driven method which is ideally suited for the study of such highly nonlinear and intermittent dynamics, but the trivial symmetries of the Rayleigh-Bénard problem such as horizontal shift-invariance can mask the interesting dynamics. To overcome this issue, the vertical velocity is averaged over parcels of similar temperature and height, which substantially compresses the size of the dataset and removes trivial horizontal symmetries. This isothermally averaged dataset, which is shown to preserve the net convective heat-flux across horizontal surfaces, is then used as an input to NLSA. The analysis generates a small number of orthogonal modes which describe the spatiotemporal variability of the heat transfer. A regression analysis shows that the extreme events of the net heat transfer are primarily associated with a family of

  13. Ocean Raman Scattering in Satellite Backscatter UV Measurements

    NASA Technical Reports Server (NTRS)

    Vasilkov, Alexander P.; Joiner, Joanna; Gleason, James; Bhartia, Pawan; Bhartia, P. K. (Technical Monitor)

    2002-01-01

    Ocean Raman scattering significantly contributes to the filling-in of solar Fraunhofer lines measured by satellite backscatter ultraviolet (buy) instruments in the cloudless atmosphere over clear ocean waters. A model accounting for this effect in buy measurements is developed and compared with observations from the Global Ozone Monitoring Experiment (GONE). The model extends existing models for ocean Raman scattering to the UV spectral range. Ocean Raman scattering radiance is propagated through the atmosphere using a concept of the Lambert equivalent reflectively and an accurate radiative transfer model for Rayleigh scattering. The model and observations can be used to evaluate laboratory measurements of pure water absorption in the UV. The good agreement between model and observations suggests that buy instruments may be useful for estimating chlorophyll content.

  14. Spin reversal and orbital torques on a viscous fluid Rayleigh sphere located arbitrarily in acoustical Bessel vortex (spiraling) beams.

    PubMed

    Mitri, F G

    2016-12-01

    The goal of this work is to demonstrate the emergence of a spin torque singularity (i.e. zero spin torque) and a spin rotation reversal of a small Rayleigh lipid/fat viscous fluid sphere located arbitrarily in space in the field of an acoustical Bessel vortex beam. This counter-intuitive property of negative spin torque generation suggests a direction of spin rotation in opposite handedness of the angular momentum carried by the incident beam. Such effects may open new capabilities in methods of quantitative characterization to determine physical properties such as viscosity, viscoelasticity, compressibility, stiffness, etc., and other techniques for the rotation and positioning using acoustical tractor beams and tweezers, invisibility cloaks, and acoustically-engineered composite metamaterials to name a few examples. Based on the descriptions for the velocity potential of the incident beam and the scattering coefficients of the sphere in the long-wavelength approximation limit, simplified expressions for the spin and orbital radiation torque components are derived. For beams with (positive or negative) unit topological charge (m=±1), the axial spin torque component for a Rayleigh absorptive sphere is maximal at the center of the beam, while it vanishes for |m|>1 therein. Moreover, the longitudinal orbital torque component, causing the sphere to rotate around the center of the beam is evaluated based on the mathematical decomposition using the gradient, scattering and absorption transverse radiation force vector components. It is shown that there is no contribution of the gradient transverse force to the orbital torque, which is only caused by the scattering and absorption transverse force components. Though the incident acoustical vortex beam carrying angular momentum causes the sphere to rotate in the same orbital direction of the beam handedness, it induces a spin torque singularity (i.e. zero spin torque) and subsequent sign reversal. This phenomenon of

  15. Atmospheric tomography with Rayleigh laser beacons for correction of wide fields and 30-m-class telescopes

    NASA Astrophysics Data System (ADS)

    Angel, J. Roger P.; Lloyd-Hart, Michael

    2000-07-01

    Single sodium beacons will likely be the most convenient for adaptive systems to correct 6 - 10 m class telescopes over a small field of view (the isoplanatic angle), provided reliable, powerful 589 nm lasers become available and affordable. However, when adaptive optics are applied to extended fields of view and correction of telescopes as large as 32 m diameter, it seems likely that laser beacons produced by Rayleigh scattering will be preferred. For these more demanding applications which require atmospheric tomography, Rayleigh beacons come into their own for two reasons. First, the cone effect, which causes the high turbulence to be sampled at a different scale, is no longer problematic when multiple lasers are used and height dependence is solved for explicitly. Second, the tomographic solution can make use of the beacon created by a laser pulse during all of its journey through the upper atmosphere, not just scattering from a thin layer selected by range gating. In this way a laser that costs an order of magnitude less to buy and maintain than a sodium laser of the same power can yield a brighter beacon and more information about the atmospheric turbulence. This is important because both the number and brightness of beacons or stars must increase with the number of layers included in the tomographic solution. For the same reason, tomography with natural stars is unlikely to be valuable for very large telescopes because in general the number and required brightness of each star increase with corrected field angle, while current narrow-field adaptive optics systems relying on natural stars are already very limited in sky coverage. Our method for tomography to take advantage of Rayleigh scattering over a wide range of heights uses short pulses from near diffraction-limited, ultraviolet lasers, projected from a small aperture above the telescope's secondary mirror. Each pulse subtends less than 1 arcsec at any instant as it travels up through many kilometers. An

  16. Schwinger-Keldysh canonical formalism for electronic Raman scattering

    NASA Astrophysics Data System (ADS)

    Su, Yuehua

    2016-03-01

    Inelastic low-energy Raman and high-energy X-ray scatterings have made great progress in instrumentation to investigate the strong electronic correlations in matter. However, theoretical study of the relevant scattering spectrum is still a challenge. In this paper, we present a Schwinger-Keldysh canonical perturbation formalism for the electronic Raman scattering, where all the resonant, non-resonant and mixed responses are considered uniformly. We show how to use this formalism to evaluate the cross section of the electronic Raman scattering off an one-band superconductor. All the two-photon scattering processes from electrons, the non-resonant charge density response, the elastic Rayleigh scattering, the fluorescence, the intrinsic energy-shift Raman scattering and the mixed response, are included. In the mean-field superconducting state, Cooper pairs contribute only to the non-resonant response. All the other responses are dominated by the single-particle excitations and are strongly suppressed due to the opening of the superconducting gap. Our formalism for the electronic Raman scattering can be easily extended to study the high-energy resonant inelastic X-ray scattering.

  17. Analysis of Raman scattered Ly-alpha emissions from the atmosphere of Uranus

    NASA Astrophysics Data System (ADS)

    Yelle, R. V.; Doose, L. R.; Tomasko, M. G.; Strobel, D. F.

    1987-05-01

    A line at 1280 Å, due to Raman scattering of solar Lyman alpha in the atmosphere of Uranus, has been detected by the Voyager Ultraviolet Spectrometer. The measured intensity of 40±20 R implies that 200 R to 500 R of the measured 1500 R Ly-α intensity at the sub-solar point is due to Rayleigh scattering of the solar line. The presence of Rayleigh and Raman scattering at 1216 Å suggests that the Uranian atmosphere is largely devoid of absorbing hydrocarbons above the 0.5 mbar level. The most natural explanation of this depletion is very weak vertical mixing equivalent to an eddy coefficient on the order of 200 cm2s-1 between 0.5 mbar and 100 mbar.

  18. Study of effective atomic number of breast tissues determined using the elastic to inelastic scattering ratio

    NASA Astrophysics Data System (ADS)

    Antoniassi, M.; Conceição, A. L. C.; Poletti, M. E.

    2011-10-01

    In this work we have measured Compton and Rayleigh scattering radiation from normal (adipose and fibroglandular), benign (fibroadenoma) and malignant (ductal carcinoma) breast tissues using a monoenergetic beam of 17.44 keV and a scattering angle of 90° ( x=0.99 Å -1). A practical method using the area of Rayleigh and Compton scattering was used for determining the effective atomic number ( Zeff) of the samples, being validated through measurements of several reference materials. The results show that there are differences in the distributions of Zeff of breast tissues, which are mainly related to the elemental composition of carbon ( Z=6) and oxygen ( Z=8) of each tissue type. The results suggest that is possible to use the method to characterize the breast tissues permitting study histological features of the breast tissues related to their elemental composition.

  19. Plasmon Mapping in Metallic Nanostructures and its Application to Single Molecule Surface Enhanced Raman Scattering: Imaging Electromagnetic Hot-Spots and Analyte Location

    SciTech Connect

    Camden, Jon P

    2013-07-16

    A major component of this proposal is to elucidate the connection between optical and electron excitation of plasmon modes in metallic nanostructures. These accomplishments are reported: developed a routine protocol for obtaining spatially resolved, low energy EELS spectra, and resonance Rayleigh scattering spectra from the same nanostructures.; correlated optical scattering spectra and plasmon maps obtained using STEM/EELS.; and imaged electromagnetic hot spots responsible for single-molecule surface-enhanced Raman scattering (SMSERS).

  20. Resonant coupling of Rayleigh waves through a narrow fluid channel causing extraordinary low acoustic transmission.

    PubMed

    Garcia-Chocano, Victor M; Nagaraj; Lòpez-Rios, Tomàs; Gumen, Lyudmila; Sànchez-Dehesa, Josè; Krokhin, Arkadii

    2012-10-01

    Coupling of Rayleigh waves propagating along two metal surfaces separated by a narrow fluid channel is predicted and experimentally observed. Although the coupling through a fluid (water) is weak, a strong synchronization in propagation of Rayleigh waves even for the metals with sufficiently high elastic contrast (brass and aluminum) is observed. Dispersion equation for two polarizations of the coupled Rayleigh waves is derived and experimentally confirmed. Excitation of coupled Rayleigh waves in a channel of finite length leads to anomalously low transmission of acoustic energy at discrete set of resonant frequencies. This effect may find useful applications in the design of acoustic metamaterial screens and reflectors.

  1. Utilization of high-frequency Rayleigh waves in near-surface geophysics

    USGS Publications Warehouse

    Xia, J.; Miller, R.D.; Park, C.B.; Ivanov, J.; Tian, G.; Chen, C.

    2004-01-01

    Shear-wave velocities can be derived from inverting the dispersive phase velocity of the surface. The multichannel analysis of surface waves (MASW) is one technique for inverting high-frequency Rayleigh waves. The process includes acquisition of high-frequency broad-band Rayleigh waves, efficient and accurate algorithms designed to extract Rayleigh-wave dispersion curves from Rayleigh waves, and stable and efficient inversion algorithms to obtain near-surface S-wave velocity profiles. MASW estimates S-wave velocity from multichannel vertical compoent data and consists of data acquisition, dispersion-curve picking, and inversion.

  2. An Instantaneous Sub-Rayleigh-to-Supershear Transition Mechanism

    NASA Astrophysics Data System (ADS)

    Liu, Y.; Lapusta, N.

    2006-12-01

    Observations suggest that supershear bursts and sustained supershear propagation may have occurred in a number of earthquakes (such as 1992 Landers, 1999 Izmit, and 2001 Kunlun). Two mechanisms have been proposed to explain the sub-Rayleigh-to supershear rupture transition. In the Burridge-Andrews mechanism (e.g., Andrews, 1976), the shear-wave stress peak traveling in front of the main Mode II rupture nucleates a daughter crack, if the prestress on the fault is large enough, and the daughter crack is born supershear. Alternatively, supershear burst can result from breaking a strong heterogeneity on a 3D fault as shown by Dunham et al. (2003). Taking a broader look at the Burridge-Andrews mechanism, we hypothesize that, for the model to produce rupture transition from sub-Rayleigh to supershear speeds, it needs to accomplish two goals: (i) nucleate a crack and (ii) drive the crack fast enough. These processes are inseparable in the Burridge-Andrews mechanism, as they both occur at the shear stress peak of the main Mode II crack propagating in a uniform prestress field. Our simulations show that goals (i) and (ii) can be achieved in other ways. For example, one can advance Mode II rupture towards a location susceptible to crack nucleation, such as a preexisting static crack, a patch of lower static frictional strength, or a patch of higher prestress. In these cases and under the right conditions, the secondary crack nucleates before the shear stress peak arrives at the nucleation site, and yet the stress field of the advancing main rupture is still able to drive the secondary crack to supershear speeds. Hence nucleating the daughter crack at the shear wave stress peak, as it is done in the Burridge- Andrews mechanism, is not essential for the subsequent supershear propagation. One can also use different means of driving the crack supershear, such as statically overstressing a part of the rupture or imposing an outside dynamic stress field. We observe the following

  3. On Lamb and Rayleigh Wave Convergence in Viscoelastic Tissues

    PubMed Central

    Nenadic, Ivan Z.; Urban, Matthew W.; Aristizabal, Sara; Mitchell, Scott A.; Humphrey, Tye C.; Greenleaf, James F.

    2012-01-01

    Characterization of the viscoelastic material properties of soft tissue has become an important area of research over the last two decades. Our group has been investigating the feasibility of using Shearwave Dispersion Ultrasound Vibrometry (SDUV) method to excite Lamb waves in organs with plate-like geometry to estimate the viscoelasticity of the medium of interest. The use of Lamb wave Dispersion Ultrasound Vibrometry (LDUV) to quantify mechanical properties of viscoelastic solids has previously been reported. Two organs, the heart wall and the spleen, can be readily modeled using plate-like geometries. The elasticity of these two organs is important because they change in pathological conditions. Diastolic dysfunction is the inability of the left ventricle (LV) of the heart to supply sufficient stroke volumes into the systemic circulation and is accompanied by the loss of compliance and stiffening of the LV myocardium. It has been shown that there is a correlation between high splenic stiffness in patients with chronic liver disease and strong correlation between spleen and liver stiffness. Here, we investigate the use of the SDUV method to quantify viscoelasticity of the LV free-wall myocardium and spleen by exciting Rayleigh waves on the organ’s surface and measuring the wave dispersion (change of wave velocity as a function of frequency) in the frequency range 40–500 Hz. An equation for Rayleigh wave dispersion due to cylindrical excitation was derived by modeling the excised myocardium and spleen with a homogenous Voigt material plate immersed in a nonviscous fluid. Boundary conditions and wave potential functions were solved for the surface wave velocity. Analytical and experimental convergence between the Lamb and Rayleigh waves is reported in a finite element model of a plate in a fluid of similar density, gelatin plate and excised porcine spleen and left-ventricular free-wall myocardium. PMID:21970846

  4. Rayleigh-Taylor instability with finite current relaxation

    NASA Astrophysics Data System (ADS)

    Silveira, F. E. M.; Orlandi, H. I.

    2016-04-01

    In this work, we explore the influence of perturbative wavelengths, shorter than those usually considered, on the growth rate of the Rayleigh-Taylor modes. Therefore, we adopt an extended form of Ohm's law which includes a finite relaxation time of the current density due to inertial effects of charged species in the plasma. The restoring force density that acts upon charged species close to the mode rational surface takes into account a new term which is usually neglected with respect to the motional electromotive force. We find that the width of the resistive layer can be interpreted in terms of the "height" of free fall in a constant gravitational field, in the Alfvén time interval. We also show that the charged species must fall "down" in the constant gravitational field in order that the static state of equilibrium of the system becomes unstable to the linear perturbation. Through the principle of conservation of energy, we find a general formula which gives the growth rate γ of the Rayleigh-Taylor modes. When the new term becomes negligible with respect to the motional electromotive force, we recover the standard result of the Rayleigh-Taylor instability, which establishes that γ scales with the plasma resistivity η as γ ˜ η 1 / 3 . However, in the opposite limiting situation, we find that γ does not depend any longer on the plasma resistivity and scales now with the electron number density n e as γ ˜ ne - 1 / 2 . Further developments of our theory may contribute to improve our understanding on the excitation mechanisms of resistive plasma instabilities by transient phenomena such as shock waves.

  5. Two-dimensional Rayleigh model of vapor bubble evolution

    SciTech Connect

    Amendt, P; Friedman, M; Glinsky, M; Gurewitz, E; London, R A; Strauss, M

    1999-01-14

    The understanding of vapor bubble generation in an aqueous tissue near a fiber tip has required advanced two dimensional (2D) hydrodynamic simulations. For 1D spherical bubble expansion a simplified and useful Rayleigh-type model can be applied. For 2D bubble evolution, such a model does not exist. The present work proposes a Rayleigh-type model for 2D bubble expansion that is faster and simpler than the 2D hydrodynamic simulations. The model is based on a flow potential representation of the hydrodynamic motion controlled by a Laplace equation and a moving boundary condition. We show that the 1D Rayleigh equation is a specific case of our model. The Laplace equation is solved for each time step by a finite element solver using a triangulation of the outside bubble region by a fast unstructured mesh generator. Two problems of vapor bubbles generated by short-pulse lasers near a fiber tip-are considered: (a) the outside region has no boundaries except the fiber, (b) the fiber and the bubble are confined in a long channel, which simulates a fiber in a vessel wall. Our simulations for problems of type (a) include features of bubble evolution as seen in experiments, including a collapse away from the fiber tip. A different behavior was obtained for problems of type (b) when the channel boundary is close to the fiber. In this case the bubble's expansion and collapse are both extremely slow in the direction normal to this boundary and distortion of the bubble is observed.

  6. Large field enhancement obtained by combining Fabry–Perot resonance and Rayleigh anomaly in photonic crystal slabs

    NASA Astrophysics Data System (ADS)

    Dossou, Kokou B.

    2017-04-01

    By applying the properties of Fabry–Perot resonance and Rayleigh anomaly, we have shown that a photonic crystal slab can scatter the light from an incident plane wave into a diffracted light with a very large reflection or transmission coefficient. The enhanced field is either a propagating diffracted wave (with a grazing angle of diffraction) or a weakly evanescent diffracted wave, so it can be particularly useful for applications requiring an enhanced propagating field (or an enhanced field with a low attenuation). An efficient effective medium technique is developed for the design of the resonant photonic crystal slabs. Numerical simulations have shown that photonic crystal slabs with low index contrast, such as the ones found in the cell wall of diatoms, can enhance the intensity of the incident light by four orders of magnitude.

  7. SH Wave Scattering from a Sinusoidal Grating

    DTIC Science & Technology

    1989-08-01

    468-471. Rayleigh , Lord (J. W. Strutt ) (1907). On the dynamical theory of gratings, Proc. Roy. Soc., Ser. A. 79, 399-416. 32 Varadan, V. K., A...version of the Rayleigh method, formulated in the wavenumber domain. However, since Lippmann (1953) questioned the expansion used in the Rayleigh method...the so called " Rayleigh ansatz", the history of this modeling approach has been shrouded in controversy. Lippmann suggested that the Rayleigh

  8. Raman scattering by H2 and N2 in the atmospheres of exoplanets

    NASA Astrophysics Data System (ADS)

    Oklopcic, Antonija; Hirata, Christopher M.; Heng, Kevin

    2016-06-01

    Rayleigh scattering is an important source of opacity in the atmospheres of exoplanets at short optical and near-UV wavelengths. Raman scattering is an inelastic process related to Rayleigh scattering, but with a weaker cross section. We analyze the signatures of Raman scattering imprinted in the reflected light and the geometric albedo of exoplanets. Raman scattering causes filling-in of absorption lines in the incident spectrum, thus producing sharp enhancements in the geometric albedo. It also shifts the wavelengths of spectral features in the reflected light causing the Raman ghost lines. Observing the albedo enhancements could be used to measure the column density of the scattering molecule and provide constrains on the presence of clouds and hazes in the atmosphere. Observing the Raman ghost lines could be used to spectroscopically identify the main scatterer in the atmosphere -- molecules like H2 or N2 which do not show prominent spectral signatures in the optical wavelength range. If detected, ghost lines could also provide information about the temperature of the atmosphere. Here we present how these signatures of Raman scattering in hydrogen- and nitrogen-dominated atmospheres can be used as probes of atmospheric pressure, temperature and composition. We analyze the feasibility of detecting these features in the albedo spectra of nearby exoplanets with the existing and future observational facilities.

  9. Rocketborne Rayleigh lidar for in situ measurements of neutral atmospheric density.

    PubMed

    Eriksen, T; Hoppe, U P; Thrane, E V; Blix, T A

    1999-04-20

    We describe the design of a small Rayleigh scattering lidar for launch on a sounding rocket as well as the first, to our knowledge, in situ measurements of neutral number density performed with a rocketborne lidar in the mesosphere. The aim of the experiment is to study the dynamics of the neutral atmosphere with emphasis on turbulent structures and gravity waves. The altitude resolution of the density profile is better than 10 m. The uncertainty is 0.3% below 55 km and better than 1% to an altitude of 65 km. The lidar technique meets the requirement of measurement of total molecular density outside the shock front surrounding the supersonic payload, which is necessary for precision measurements of neutral atmospheric density. We have compared different component technologies and design approaches and show performance calculations for two electro-optical systems. The first system has laser and detector components that were available in 1993, the second has new solutions that became available in 1995. The second system has a signal-to-noise ratio that is five times higher than the first and employs a pulsed high-power laser diode array as the transmitter and a large-area avalanche photodiode as the receiver.

  10. Nonlinear Evolution of Rayleigh-Taylor Instability in a Radiation-supported Atmosphere

    NASA Astrophysics Data System (ADS)

    Jiang, Yan-Fei; Davis, Shane W.; Stone, James M.

    2013-02-01

    The nonlinear regime of Rayleigh-Taylor instability (RTI) in a radiation supported atmosphere, consisting of two uniform fluids with different densities, is studied numerically. We perform simulations using our recently developed numerical algorithm for multi-dimensional radiation hydrodynamics based on a variable Eddington tensor (VET) as implemented in Athena, focusing on the regime where scattering opacity greatly exceeds absorption opacity. We find that the radiation field can reduce the growth and mixing rate of RTI, but this reduction is only significant when radiation pressure significantly exceeds gas pressure. Small-scale structures are also suppressed in this case. In the nonlinear regime, dense fingers sink faster than rarefied bubbles can rise, leading to asymmetric structures about the interface. By comparing the calculations that use a VET versus the Eddington approximation, we demonstrate that anisotropy in the radiation field can affect the nonlinear development of RTI significantly. We also examine the disruption of a shell of cold gas being accelerated by strong radiation pressure, motivated by models of radiation driven outflows in ultraluminous infrared galaxies. We find that when the growth timescale of RTI is smaller than acceleration timescale, the amount of gas that would be pushed away by the radiation field is reduced due to RTI.

  11. NONLINEAR EVOLUTION OF RAYLEIGH-TAYLOR INSTABILITY IN A RADIATION-SUPPORTED ATMOSPHERE

    SciTech Connect

    Jiang, Yan-Fei; Stone, James M.; Davis, Shane W.

    2013-02-15

    The nonlinear regime of Rayleigh-Taylor instability (RTI) in a radiation supported atmosphere, consisting of two uniform fluids with different densities, is studied numerically. We perform simulations using our recently developed numerical algorithm for multi-dimensional radiation hydrodynamics based on a variable Eddington tensor (VET) as implemented in Athena, focusing on the regime where scattering opacity greatly exceeds absorption opacity. We find that the radiation field can reduce the growth and mixing rate of RTI, but this reduction is only significant when radiation pressure significantly exceeds gas pressure. Small-scale structures are also suppressed in this case. In the nonlinear regime, dense fingers sink faster than rarefied bubbles can rise, leading to asymmetric structures about the interface. By comparing the calculations that use a VET versus the Eddington approximation, we demonstrate that anisotropy in the radiation field can affect the nonlinear development of RTI significantly. We also examine the disruption of a shell of cold gas being accelerated by strong radiation pressure, motivated by models of radiation driven outflows in ultraluminous infrared galaxies. We find that when the growth timescale of RTI is smaller than acceleration timescale, the amount of gas that would be pushed away by the radiation field is reduced due to RTI.

  12. Bubble Counts for Rayleigh-Taylor Instability Using Image Analysis

    SciTech Connect

    Miller, P L; Gezahegne, A G; Cook, A W; Cabot, W H; Kamath, C

    2007-01-24

    We describe the use of image analysis to count bubbles in 3-D, large-scale, LES [1] and DNS [2] of the Rayleigh-Taylor instability. We analyze these massive datasets by first converting the 3-D data to 2-D, then counting the bubbles in the 2-D data. Our plots for the bubble count indicate there are four distinct regimes in the process of the mixing of the two fluids. We also show that our results are relatively insensitive to the choice of parameters in our analysis algorithms.

  13. Stellar convection 3: Convection at large Rayleigh numbers

    NASA Technical Reports Server (NTRS)

    Marcus, P. S.

    1979-01-01

    A three dimensional study of convection in a self gravitating sphere of Boussinesq fluid with a Rayleigh number of 10 to the 10th power and a Prandtl of 1 is presented. The velocity and temperature of the fluid are computed at the largest wavelengths using spectral methods. A confirmation that the fluid is anisotropic and that the energy spectra are not smooth functions of wavelength but have a large amount of fine structure is discussed. The parameterization of the transport properties of the unresolvable inertial subrange with eddy viscosities and diffusivities is described. The time dependent fluctuations in the energy spectra and how they cascade from large to small wavelengths is examined.

  14. Rayleigh-Taylor instability in quantum magnetized viscous plasma

    SciTech Connect

    Hoshoudy, G. A.

    2011-09-15

    Quantum effects on Rayleigh-Taylor instability of stratified viscous plasmas layer under the influence of vertical magnetic field are investigated. By linearly solving the viscous QMHD equations into normal mode, a forth-order ordinary differential equation is obtained to describe the velocity perturbation. Then the growth rate is derived for the case where a plasma with exponential density distribution is confined between two rigid planes. The results show that, the presence of vertical magnetic field beside the quantum effect will bring about more stability on the growth rate of unstable configuration for viscous plasma, which is greater than that of inviscous plasma.

  15. Selective Manipulation of Microscopic Particles with Precursor Swirling Rayleigh Waves

    NASA Astrophysics Data System (ADS)

    Riaud, Antoine; Baudoin, Michael; Bou Matar, Olivier; Becerra, Loic; Thomas, Jean-Louis

    2017-02-01

    Contactless manipulation of microparticles is demonstrated with single-beam acoustical tweezers based on precursor swirling Rayleigh waves. These surface waves degenerate into acoustical vortices when crossing a stack made of a fluid layer and its solid support, hence creating a localized acoustical trap in a fluid cavity. They can be synthesized with a single interdigitated transducer whose spiraling shape encodes the phase of the field like a hologram. For applications, these tweezers have many attractive features: they are selective, flat, easily integrable, and compatible with disposable substrates.

  16. Theoretical and Experimental Studies of Magneto-Rayleigh-Taylor Instabilities

    SciTech Connect

    Lau, Yue Ying; Gilgenbach, Ronald

    2013-07-07

    Magneto-Rayleigh-Taylor instability (MRT) is important to magnetized target fusion, wire-array z-pinches, and equation-of-state studies using flyer plates or isentropic compression. It is also important to the study of the crab nebula. The investigators performed MRT experiments on thin foils, driven by the mega-ampere linear transformer driver (LTD) facility completed in their laboratory. This is the first 1-MA LTD in the USA. Initial experiments on the seeding of MRT were performed. Also completed was an analytic study of MRT for a finite plasma slab with arbitrary magnetic fields tangential to the interfaces. The effects of magnetic shear and feedthrough were analyzed.

  17. Ultrasonic characterization of functionally gradient materials with leaky Rayleigh wave

    SciTech Connect

    Kawashima, Koichiro; Takenouchi, Naoki; Awaji, Hideo; Nishikawa, Tadahiro

    1999-12-02

    Young's modulus of functionally gradient Al{sub 2}O{sub 3}/Ni ceramics, which was formed by centrifugal casting and has gradient of the elastic properties along a particular direction on the surface, is estimated by velocity measurement of the leaky Rayleigh and longitudinal waves. Those velocities were measured every 1mm with a line focused PVDF transducer, of which central frequency, focal length and width are 36MHz, 5mm and 8mm. Thus measured Young's modulus varies from 370GPa (Al{sub 2}O{sub 3} rich side) to 200GPa (Ni rich side)

  18. Coexisting attractors in compressible Rayleigh-Bénard flow

    NASA Astrophysics Data System (ADS)

    Castillo, V. M.; Hoover, Wm. G.; Hoover, C. G.

    1997-05-01

    We demonstrate that precise solutions of the convective flow equations for a compressible conducting viscous fluid can give degenerate stationary states. That is, two or more completely different stable flows can result for fixed stationary boundary conditions. We characterize these complex flows with finite-difference, smooth-particle methods, and high-order implicit methods. The fluids treated here are viscous conducting gases, enclosed by thermal boundaries in a gravitational field-the ``Rayleigh-Bénard problem.'' Degenerate solutions occur in both two- and three-dimensional simulations. This coexistence of solutions is a macroscopic manifestation of the strange attractors seen in atomistic systems far from equilibrium.

  19. Statistical approach of weakly nonlinear ablative Rayleigh-Taylor instability

    SciTech Connect

    Garnier, J.; Masse, L.

    2005-06-15

    A weakly nonlinear model is proposed for the Rayleigh-Taylor instability in presence of ablation and thermal transport. The nonlinear effects for a single-mode disturbance are computed, included the nonlinear correction to the exponential growth of the fundamental modulation. Mode coupling in the spectrum of a multimode disturbance is thoroughly analyzed by a statistical approach. The exponential growth of the linear regime is shown to be reduced by the nonlinear mode coupling. The saturation amplitude is around 0.1{lambda} for long wavelengths, but higher for short instable wavelengths in the ablative regime.

  20. Rayleigh-Brillouin spectrum in special relativistic hydrodynamics

    SciTech Connect

    Garcia-Perciante, A. L.; Garcia-Colin, L. S.

    2009-06-15

    In this paper we calculate the Rayleigh-Brillouin spectrum for a relativistic simple fluid according to three different versions available for a relativistic approach to nonequilibrium thermodynamics. An outcome of these calculations is that Eckart's version predicts that such spectrum does not exist. This provides an argument to question its validity. The remaining two results, which differ one from another, do provide a finite form for such spectrum. This raises the rather intriguing question as to which of the two theories is a better candidate to be taken as a possible version of relativistic nonequilibrium thermodynamics. The answer will clearly require deeper examination of this problem.

  1. Similarity relations for anisotropic scattering in absorbing media

    NASA Astrophysics Data System (ADS)

    Graaff, Reindert; Aarnoudse, Jan G.; de Mul, Frits F.; Jentink, Henk W.

    1993-02-01

    The validity of the similarity parameter (Sigma) 's equalsV (Sigma) s (1 - g), the reduced scattering coefficient, where g is the average cosine of the scattering phase function is investigated. Attenuation coefficients (alpha) and diffusion patterns are obtained from solutions of the transport equation for isotropic scattering and Rayleigh-Gans scattering, applied to infinite media. Similarity is studied for the attenuation coefficient (alpha) , as well as for the Kubelka-Munk absorption and backscattering coefficients in the positive and negative directions, and for predictions of the internal reflection at interfaces. Similarity between solutions of the Boltzmann equation for highly forward scattering and isotropic scattering (g equals 0) exist only when (Sigma) a << (Sigma) s (1 - g). However, because similarity between results, both with g > 0.9, is independent of the value of the absorption coefficient, it is advantageous to simulate highly forward scattering media like biological tissues with g > 0.9, e.g., by Monte Carlo simulations, instead of using isotropic scattering or diffusion theory. Monte Carlo simulations on slabs confirm the deviations from the diffusion approximation and show the behavior near boundaries. Application of similarity may save calculation time in Monte Carlo simulations, because simulation with a lower value for g will increase the mean free path.

  2. Dynamic Tensile Cracking in Slopes and the Possible Existence of Seismic Rayleigh Waves in a High Frequency Range

    NASA Astrophysics Data System (ADS)

    Uenishi, K.

    2011-12-01

    that the superimposition of the reflected and incident Rayleigh waves can induce large (tensile) stress amplification near the edge and thus produce crack openings in the top surface at a particular position, and for the Sendai case, considering the slope inclination angle (75 degrees) and the position of cracks (6 meters from the edge), the dominant frequency may be some 10 Hz. Although the attenuation of Rayleigh waves with travel distance is smaller than that of body waves, the existence of the estimated 10 Hz in fill slopes situated over 100 km away from the epicenter might be questionable. However, the Sendai region is historically known as one of the places where the subducting Pacific Plate acts as an efficient waveguide for high-frequency signals and these high frequencies may be transmitted to the surface through the scattering by heterogeneities in the plate structure. The velocity response spectra obtained from the 1978 and 2011 events also seem to support the idea that high-frequency seismic waves (and hence the possible conversion of body waves into Rayleigh waves in the high frequency range) did exist in the city of Sendai during the 1978 and 2011 earthquakes.

  3. Infrared (10.6-mum) scattering and extinction in laboratory water and ice clouds.

    PubMed

    Sassen, K

    1981-01-15

    Measurements of the angular scattering and extinction of IR (10.6-mum) laser radiation in laboratory water and ice clouds are reported and compared to theoretical predictions for spheres and visible (0.633-mum) light scattering data. Randomly oriented cloud particles with dimensions ranging from several times smaller to larger than the incident wavelength generated phase functions span the Rayleigh and Mie scattering domains and illustrate the effects caused by strong internal energy absorption. Dual-wavelength extinction measurements reveal information on the growth and dissipation of laboratory water clouds and the effects of cloud seeding. The remote sensing significance of the findings is discussed.

  4. Scattering intensities for a white beam (120 kV) presenting a semi-empirical model to preview scattered beams

    NASA Astrophysics Data System (ADS)

    Gonçalves, O. D.; Boldt, S.; Kasch, K. U.

    2016-09-01

    This work aims at measuring the scattering cross sections for white beams and the verification of a semi-empirical model predicting scattered energy spectra of an X-ray beam produced by an industrial X-ray tube (Pantack Sievert, 120 kV, tungsten target) incident on a water sample. Both, theoretical and semi-empirical results presented are based on the form factor approach with results well corresponding to performed measurements. The elastic (Rayleigh) scattering cross sections are based on Thomson scattering with a form factor correction as published by Morin (1982). The inelastic (Compton) contribution is based on the Klein Nishina equation (Klein and Nishina, 1929) multiplied by the incoherent scattering factors calculated by Hubbel et al. (1975). Two major results are presented: first, the experimental integrated in energy cross sections corresponds with theoretical cross sections obtained at the mean energy of the measured scattered spectra at a given angle. Secondly, the measured scattered spectra at a given angle correspond to those obtained utilizing the semi-empirical model as proposed here. A good correspondence of experimental results and model predictions can be shown. The latter, therefore, proves to be a useful method to calculate the scattering contributions in a number of applications as for example cone beam tomography.

  5. From steady solutions to chaotic flows in a Rayleigh-Bénard problem at moderate Rayleigh numbers

    NASA Astrophysics Data System (ADS)

    Puigjaner, D.; Herrero, J.; Simó, C.; Giralt, F.

    2011-05-01

    The dynamics of a Rayleigh-Bénard convection problem in a cubical cavity at moderate values of the Rayleigh number ( Ra≤105) and a Prandtl number of Pr=0.71 (with extensions to Pr=0.75 and 0.80) was investigated. The cubical cavity was heated from below and had perfectly conducting sidewalls and uniform temperature distributions on the two horizontal walls. A system of ordinary differential equations with a dimension of typically N≈11 000 was obtained when the conservation equations were discretized by means of a Galerkin method. Previous knowledge of the bifurcation diagram of steady solutions, reported in the literature, was used to identify the origin of several branches of periodic orbits that were continued with Ra. Half a dozen of such periodic orbits were found to be stable within narrow ranges of Ra (at most, some 5000 units wide). An attracting two-torus, restricted to a very narrow region of Ra, was also identified. It was found that the instabilization of periodic orbits quite often resulted into the development of complex dynamics such as the creation of homoclinic and heteroclinic orbits. Instances of both types of global bifurcations were analyzed in some detail. One particular instance of chaotic dynamics (a strange attractor) was also identified. Chaotic dynamics has been found at Pr=0.71 in a flow invariant subspace, which can be interpreted as a fixed-point subspace in terms of equivariant theory; this subspace is not attracting. However, some regions of attracting chaotic dynamics for moderate Rayleigh numbers ( 9×104≤Ra≤105) were found at values of Pr slightly above 0.71. The role of a particular homoclinic solution found at Pr=0.71 in the generation of these chaotic regions was analyzed.

  6. Effects of Rotation on a Large Rayleigh Number Bridgman Furnace

    NASA Astrophysics Data System (ADS)

    Foster, M. R.

    1998-11-01

    It is known that rotating a Bridgman furnace in a centrifuge improves the crystal quality at large Rayleigh number(W.Weber, G. Neumann & G. Mddot u)ller, J. Crys. Growth 100, 145 (1990). Here we determine improvements achieved by rotating the ampoule about its vertical axis. We know that, in the absence of rotation, if the Rayleigh number, Ra, is large and Biot number is small, much larger solutal variations in the crystal are produced by azimuthal variations in the side-wall heating than from the axisymmetric component. However, at moderately large Taylor numbers, the first effects are to reduce the helical variation in solute concentration by inhibiting vertical motion in the melt, and so for Taylor numbers larger than O(Ra^1/6), the melt convection due to axisymmetric heating produces the larger solutal variation than that from azimuthal variations. As the Taylor number increases, the helical component of material segregation continues to decline in magnitude. However, in spite of changes in the interfacial boundary layer for Taylor numbers of order Ra^1/3 and larger, the outer flow/boundary layer coupling is unaltered for axisymmetry. It is not until the Taylor number is O(Ra^1/2) that the axisymmetric flow undergoes a change sufficiently dramatic to allow significant reduction in the material segregation from the zero-rotation case.

  7. Heat transport measurements in turbulent rotating Rayleigh-Benard convection

    SciTech Connect

    Ecke, Robert E; Liu, Yuanming

    2008-01-01

    We present experimental heat transport measurements of turbulent Rayleigh-Benard convection with rotation about a vertical axis. The fluid, water with Prandtl number ({sigma}) about 6, was confined in a cell which had a square cross section of 7.3 cm x 7.3 cm and a height of 9.4 cm. Heat transport was measured for Rayleigh numbers 2 x 10{sup 5} < Ra < 5 x 10{sup 8} and Taylor numbers 0 < Ta < 5 x 10{sup 9}. We show the variation of normalized heat transport, the Nusselt number, at fixed dimensional rotation rate {Omega}{sub D}, at fixed Ra varying Ta, at fixed Ta varying Ra, and at fixed Rossby number Ro. The scaling of heat transport in the range 10{sup 7} to about 10{sup 9} is roughly 0.29 with a Ro dependent coefficient or equivalently is also well fit by a combination of power laws of the form a Ra{sup 1/5} + b Ra{sup 1/3} . The range of Ra is not sufficient to differentiate single power law or combined power law scaling. The overall impact of rotation on heat transport in turbulent convection is assessed.

  8. Rayleigh-Taylor mixing with space-dependent acceleration

    NASA Astrophysics Data System (ADS)

    Abarzhi, Snezhana

    2016-11-01

    We extend the momentum model to describe Rayleigh-Taylor (RT) mixing driven by a space-dependent acceleration. The acceleration is a power-law function of space coordinate, similarly to astrophysical and plasma fusion applications. In RT flow the dynamics of a fluid parcel is driven by a balance per unit mass of the rates of momentum gain and loss. We find analytical solutions in the cases of balanced and imbalanced gains and losses, and identify their dependence on the acceleration exponent. The existence is shown of two typical sub-regimes of self-similar RT mixing - the acceleration-driven Rayleigh-Taylor-type mixing and dissipation-driven Richtymer-Meshkov-type mixing with the latter being in general non-universal. Possible scenarios are proposed for transitions from the balanced dynamics to the imbalanced self-similar dynamics. Scaling and correlations properties of RT mixing are studied on the basis of dimensional analysis. Departures are outlined of RT dynamics with space-dependent acceleration from canonical cases of homogeneous turbulence as well as blast waves with first and second kind self-similarity. The work is supported by the US National Science Foundation.

  9. Rayleigh-Taylor mixing with time-dependent acceleration

    NASA Astrophysics Data System (ADS)

    Abarzhi, Snezhana

    2016-10-01

    We extend the momentum model to describe Rayleigh-Taylor (RT) mixing driven by a time-dependent acceleration. The acceleration is a power-law function of time, similarly to astrophysical and plasma fusion applications. In RT flow the dynamics of a fluid parcel is driven by a balance per unit mass of the rates of momentum gain and loss. We find analytical solutions in the cases of balanced and imbalanced gains and losses, and identify their dependence on the acceleration exponent. The existence is shown of two typical regimes of self-similar RT mixing-acceleration-driven Rayleigh-Taylor-type and dissipation-driven Richtymer-Meshkov-type with the latter being in general non-universal. Possible scenarios are proposed for transitions from the balanced dynamics to the imbalanced self-similar dynamics. Scaling and correlations properties of RT mixing are studied on the basis of dimensional analysis. Departures are outlined of RT dynamics with time-dependent acceleration from canonical cases of homogeneous turbulence as well as blast waves with first and second kind self-similarity. The work is supported by the US National Science Foundation.

  10. Rotating thermal convection at very large Rayleigh numbers

    NASA Astrophysics Data System (ADS)

    Weiss, Stephan; van Gils, Dennis; Ahlers, Guenter; Bodenschatz, Eberhard

    2016-11-01

    The large scale thermal convection systems in geo- and astrophysics are usually influenced by Coriolis forces caused by the rotation of their celestial bodies. To better understand the influence of rotation on the convective flow field and the heat transport at these conditions, we study Rayleigh-Bénard convection, using pressurized sulfur hexaflouride (SF6) at up to 19 bars in a cylinder of diameter D=1.12 m and a height of L=2.24 m. The gas is heated from below and cooled from above and the convection cell sits on a rotating table inside a large pressure vessel (the "Uboot of Göttingen"). With this setup Rayleigh numbers of up to Ra =1015 can be reached, while Ekman numbers as low as Ek =10-8 are possible. The Prandtl number in these experiment is kept constant at Pr = 0 . 8 . We report on heat flux measurements (expressed by the Nusselt number Nu) as well as measurements from more than 150 temperature probes inside the flow. We thank the Deutsche Forschungsgemeinschaft (DFG) for financial support through SFB963: "Astrophysical Flow Instabilities and Turbulence". The work of GA was supported in part by the US National Science Foundation through Grant DMR11-58514.

  11. Rayleigh wave inversion using heat-bath simulated annealing algorithm

    NASA Astrophysics Data System (ADS)

    Lu, Yongxu; Peng, Suping; Du, Wenfeng; Zhang, Xiaoyang; Ma, Zhenyuan; Lin, Peng

    2016-11-01

    The dispersion of Rayleigh waves can be used to obtain near-surface shear (S)-wave velocity profiles. This is performed mainly by inversion of the phase velocity dispersion curves, which has been proven to be a highly nonlinear and multimodal problem, and it is unsuitable to use local search methods (LSMs) as the inversion algorithm. In this study, a new strategy is proposed based on a variant of simulated annealing (SA) algorithm. SA, which simulates the annealing procedure of crystalline solids in nature, is one of the global search methods (GSMs). There are many variants of SA, most of which contain two steps: the perturbation of model and the Metropolis-criterion-based acceptance of the new model. In this paper we propose a one-step SA variant known as heat-bath SA. To test the performance of the heat-bath SA, two models are created. Both noise-free and noisy synthetic data are generated. Levenberg-Marquardt (LM) algorithm and a variant of SA, known as the fast simulated annealing (FSA) algorithm, are also adopted for comparison. The inverted results of the synthetic data show that the heat-bath SA algorithm is a reasonable choice for Rayleigh wave dispersion curve inversion. Finally, a real-world inversion example from a coal mine in northwestern China is shown, which proves that the scheme we propose is applicable.

  12. Shearing box simulations in the Rayleigh unstable regime

    NASA Astrophysics Data System (ADS)

    Nauman, Farrukh; Blackman, Eric G.

    2017-01-01

    We study the stability properties of Rayleigh unstable flows both in the purely hydrodynamic and magnetohydrodynamic (MHD) regimes for two different values of the shear q = 2.1, 4.2 (q = -dln Ω/dln r) and compare it with the Keplerian case q = 1.5. We find that the q > 2 regime is unstable both in the hydrodynamic and in the MHD limit (with an initially weak magnetic field). In this regime, the velocity fluctuations dominate the magnetic fluctuations. In contrast, in the q < 2 (magnetorotational instability (MRI)) regime the magnetic fluctuations dominate. This highlights two different paths to MHD turbulence implied by the two regimes, suggesting that in the q > 2 regime the instability produces primarily velocity fluctuations that cause magnetic fluctuations, with the causality reversed for the q < 2 MRI unstable regime. We also find that the magnetic field correlation is increasingly localized as the shear is increased in the Rayleigh unstable regime. In calculating the time evolution of spatial averages of different terms in the MHD equations, we find that the q > 2 regime is dominated by terms which are nonlinear in the fluctuations, whereas for q < 2, the linear terms play a more significant role.

  13. Rayleigh-Taylor instability of viscous fluids with phase change.

    PubMed

    Kim, Byoung Jae; Kim, Kyung Doo

    2016-04-01

    Film boiling on a horizontal surface is a typical example of the Rayleigh-Taylor instability. During the film boiling, phase changes take place at the interface, and thus heat and mass transfer must be taken into consideration in the stability analysis. Moreover, since the vapor layer is not quite thick, a viscous flow must be analyzed. Existing studies assumed equal kinematic viscosities of two fluids, and/or considered thin viscous fluids. The purpose of this study is to derive the analytical dispersion relation of the Rayleigh-Taylor instability for more general conditions. The two fluids have different properties. The thickness of the vapor layer is finite, but the liquid layer is thick enough to be nearly semi-infinite in view of perturbation. Initially, the vapor is in equilibrium with the liquid at the interface, and the direction of heat transfer is from the vapor side to the liquid side. In this case, the phase change has a stabilizing effect on the growth rate of the interface. When the vapor layer is thin, there is a coupled effect of the vapor viscosity, phase change, and vapor thickness on the critical wave number. For the other limit of a thick vapor, both the liquid and vapor viscosities influence the critical wave number. Finally, the most unstable wavelength is investigated. When the vapor layer is thin, the most unstable wavelength is not affected by phase change. When the vapor layer is thick, however, it increases with the increasing rate of phase change.

  14. Experimental and theoretical study of Rayleigh-Lamb wave propagation

    NASA Technical Reports Server (NTRS)

    Rogers, Wayne P.; Datta, Subhendu K.; Ju, T. H.

    1990-01-01

    Many space structures, such as the Space Station Freedom, contain critical thin-walled components. The structural integrity of thin-walled plates and shells can be monitored effectively using acoustic emission and ultrasonic testing in the Rayleigh-Lamb wave frequency range. A new PVDF piezoelectric sensor has been developed that is well suited to remote, inservice nondestructive evaluation of space structures. In the present study the new sensor was used to investigate Rayleigh-Lamb wave propagation in a plate. The experimental apparatus consisted of a glass plate (2.3 m x 25.4 mm x 5.6 mm) with PVDF sensor (3 mm diam.) mounted at various positions along its length. A steel ball impact served as a simulated acoustic emission source, producing surface waves, shear waves and longitudinal waves with dominant frequencies between 1 kHz and 200 kHz. The experimental time domain wave-forms were compared with theoretical predictions of the wave propagation in the plate. The model uses an analytical solution for the Green's function and the measured response at a single position to predict response at any other position in the plate. Close agreement was found between the experimental and theoretical results.

  15. Wind reversals in turbulent Rayleigh-Bénard convection.

    PubMed

    Araujo, Francisco Fontenele; Grossmann, Siegfried; Lohse, Detlef

    2005-08-19

    The phenomenon of irregular cessation and subsequent reversal of the large-scale circulation in turbulent Rayleigh-Bénard convection is theoretically analyzed. The force and thermal balance on a single plume detached from the thermal boundary layer yields a set of coupled nonlinear equations, whose dynamics is related to the Lorenz equations. For Prandtl and Rayleigh numbers in the range 10(-2) < or = Pr < or = 10(3) and 10(7) < or = Ra < or = 10(12), the model has the following features: (i) chaotic reversals may be exhibited at Ra > or = 10(7); (ii) the Reynolds number based on the root mean square velocity scales as Re(rms) approximately Ra([0.41...0.47]) (depending on Pr), and as Re(rms) approximately Pr(-[0.66...0.76]) (depending on Ra); and (iii) the mean reversal frequency follows an effective scaling law omega/(nu L(-2)) approximately Pr(-(0.64 +/- 0.01))Ra(0.44 +/- 0.01). The phase diagram of the model is sketched, and the observed transitions are discussed.

  16. Instability vaccination: A structural design to reduce Rayleigh Taylor instability

    NASA Astrophysics Data System (ADS)

    Esmaeili, Amin

    2013-10-01

    Instability vaccination can be defined as designing a structure to stimulate the system in order to develop immunity against its instability. In this work we have tried to do this stabilization by a new technique. Previously some suppression of R-M instability was done by insertion of magnetic field, but in this work we have tried to do this suppression by proposing a configuration similar to the shape of instability, we call it instability vaccination. This design will reduce the rotations (mostly rotations of Rayleigh Taylor instability) in the fluids that cause more mixing and instabilities. In this paper, we consider the evolution of the interface between two ideal semi-infinite fluid surfaces, using two-dimensional Riemann solver, to solve the Euler equations. First, we performed evolution of a rectangular disorder between the 2 surfaces using two-dimensional Riemann problem for the equations of Euler. Next, the interface was replaced with a perturbation that was part rectangular and part semi-circular (like a mushroom). The simulation was continued till some time steps using the HLL method. We have seen that the rotations of Rayleigh Taylor (R-T) instability were decreased in the second case. Email: amin@cavelab.cs.tsukuba.ac.jp

  17. Non-linear characteristics of Rayleigh-Taylor instable perturbations

    NASA Astrophysics Data System (ADS)

    Fan, Zhengfeng; Luo, Jisheng

    2008-04-01

    The direct numerical simulation method is adopted to study the non-linear characteristics of Rayleigh-Taylor instable perturbations at the ablation front of a 200 μm planar CH ablation target. In the simulation, the classical electrical thermal conductivity is included, and NND difference scheme is used. The linear growth rates obtained from the simulation agree with the Takabe formula. The amplitude distribution of the density perturbation at the ablation front is obtained for the linear growth case. The non-linear characteristics of Rayleigh-Taylor instable perturbations are analyzed and the numerical results show that the amplitude distributions of the compulsive harmonics are very different from that of the fundamental perturbation. The characteristics of the amplitude distributions of the harmonics and their fast growth explain why spikes occur at the ablation front. The numerical results also show that non-linear effects have relations with the phase differences of double mode initial perturbations, and different phase differences lead to varied spikes.

  18. The Inhibition of the Rayleigh-Taylor Instability by Rotation.

    PubMed

    Baldwin, Kyle A; Scase, Matthew M; Hill, Richard J A

    2015-07-01

    It is well-established that the Coriolis force that acts on fluid in a rotating system can act to stabilise otherwise unstable flows. Chandrasekhar considered theoretically the effect of the Coriolis force on the Rayleigh-Taylor instability, which occurs at the interface between a dense fluid lying on top of a lighter fluid under gravity, concluding that rotation alone could not stabilise this system indefinitely. Recent numerical work suggests that rotation may, nevertheless, slow the growth of the instability. Experimental verification of these results using standard techniques is problematic, owing to the practical difficulty in establishing the initial conditions. Here, we present a new experimental technique for studying the Rayleigh-Taylor instability under rotation that side-steps the problems encountered with standard techniques by using a strong magnetic field to destabilize an otherwise stable system. We find that rotation about an axis normal to the interface acts to retard the growth rate of the instability and stabilise long wavelength modes; the scale of the observed structures decreases with increasing rotation rate, asymptoting to a minimum wavelength controlled by viscosity. We present a critical rotation rate, dependent on Atwood number and the aspect ratio of the system, for stabilising the most unstable mode.

  19. Experimental Study of Rayleigh-Taylor Instability Using Paramagnetic Fluids

    NASA Astrophysics Data System (ADS)

    Tsiklashvili, Vladimer; Likhachev, Oleg; Jacobs, Jeffry

    2009-11-01

    Experiments that take advantage of the properties of paramagnetic liquids are used to study Rayleigh-Taylor instability. A gravitationally unstable combination of a paramagnetic salt solution and a nonmagnetic solution is initially stabilized by a magnetic field gradient that is produced by the contoured pole-caps of a large electromagnet. Rayleigh-Taylor instability originates with the rapid removal of current from the electromagnet, which results in the heavy liquid falling into the light liquid due to gravity and, thus, mixing with it. The mixing zone is visualized by back-lit photography and is recorded with a digital video camera. For visualization purposes, a blue-green dye is added to the magnetic fluid. The mixing rate of the two liquids is determined from an averaged dye concentration across the mixing layer by means of the Beer-Lambert law. After removal of the suspending magnetic field, the initially flat interface between the two liquids develops a random surface pattern with the dominant length scale well approximated by the fastest growing wavelength in accordance with the viscous linear stability theory. Several combinations of paramagnetic and nonmagnetic solutions have been considered during the course of the research. A functional dependence of the mixing layer growth constant, α, on the properties of the liquids is a primary subject of the present study.

  20. The Inhibition of the Rayleigh-Taylor Instability by Rotation

    PubMed Central

    Baldwin, Kyle A.; Scase, Matthew M.; Hill, Richard J. A.

    2015-01-01

    It is well-established that the Coriolis force that acts on fluid in a rotating system can act to stabilise otherwise unstable flows. Chandrasekhar considered theoretically the effect of the Coriolis force on the Rayleigh-Taylor instability, which occurs at the interface between a dense fluid lying on top of a lighter fluid under gravity, concluding that rotation alone could not stabilise this system indefinitely. Recent numerical work suggests that rotation may, nevertheless, slow the growth of the instability. Experimental verification of these results using standard techniques is problematic, owing to the practical difficulty in establishing the initial conditions. Here, we present a new experimental technique for studying the Rayleigh-Taylor instability under rotation that side-steps the problems encountered with standard techniques by using a strong magnetic field to destabilize an otherwise stable system. We find that rotation about an axis normal to the interface acts to retard the growth rate of the instability and stabilise long wavelength modes; the scale of the observed structures decreases with increasing rotation rate, asymptoting to a minimum wavelength controlled by viscosity. We present a critical rotation rate, dependent on Atwood number and the aspect ratio of the system, for stabilising the most unstable mode. PMID:26130005