Synthesis of rutherfordium isotopes in the 238U(26Mg, xn)264-xRf reaction and study of their decay properties

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gates, Jacklyn M; Gates, J.M.; Garcia, M.A.

2008-01-15

Isotopes of rutherfordium (258-261Rf) were produced in irradiations of 238U targets with 26Mg beams. Excitation functions were measured for the 4n, 5n and 6n exit channels. Production of 261Rf in the 3n exit channel with a cross section of 28+92-26 pb was observed. Alpha decay of 258Rf was observed for the first time with an alpha-particle energy of 9.05+-0.03 MeV and an alpha/total decay branching ratio of 0.31+-0.11. In 259Rf, the electron capture/total decay branching ratio was measured to be 0.15+-0.04. The measured half-lives for 258Rf, 259Rf and 260Rf were 14.7+1.2-1.0 ms, 2.5+0.4-0.3 s and 22.2+3.0-2.4 ms, respectively, in agreementmore » with literature data. The systematics of the alpha decay Q values and of the partial spontaneous fission half-lives were evaluated for even-even nuclides in the region of the N = 152, Z = 100 deformed shell. The influence of the N = 152 shell on the alpha decay Q values for rutherfordium was observed to be similar to that of the lighter elements (96<_ Z<_ 102). However, the N = 152 shell does not stabilize the rutherfordium isotopes against spontaneous fission, as it does in the lighter elements (96<_ Z<_102).« less

The recoil transfer chamber—An interface to connect the physical preseparator TASCA with chemistry and counting setups

NASA Astrophysics Data System (ADS)

Even, J.; Ballof, J.; Brüchle, W.; Buda, R. A.; Düllmann, Ch. E.; Eberhardt, K.; Gorshkov, A.; Gromm, E.; Hild, D.; Jäger, E.; Khuyagbaatar, J.; Kratz, J. V.; Krier, J.; Liebe, D.; Mendel, M.; Nayak, D.; Opel, K.; Omtvedt, J. P.; Reichert, P.; Runke, J.; Sabelnikov, A.; Samadani, F.; Schädel, M.; Schausten, B.; Scheid, N.; Schimpf, E.; Semchenkov, A.; Thörle-Pospiech, P.; Toyoshima, A.; Türler, A.; Vicente Vilas, V.; Wiehl, N.; Wunderlich, T.; Yakushev, A.

2011-05-01

Performing experiments with transactinide elements demands highly sensitive detection methods due to the extremely low production rates (one -atom -at -a -time conditions). Preseparation with a physical recoil separator is a powerful method to significantly reduce the background in experiments with sufficiently long-lived isotopes ( t1/2≥0.5 s). In the last years, the new gas-filled TransActinide Separator and Chemistry Apparatus (TASCA) was installed and successfully commissioned at GSI. Here, we report on the design and performance of a Recoil Transfer Chamber (RTC) for TASCA—an interface to connect various chemistry and counting setups with the separator. Nuclear reaction products recoiling out of the target are separated according to their magnetic rigidity within TASCA, and the wanted products are guided to the focal plane of TASCA. In the focal plane, they pass a thin Mylar window that separates the ˜1 mbar atmosphere in TASCA from the RTC kept at ˜1 bar. The ions are stopped in the RTC and transported by a continuous gas flow from the RTC to the ancillary setup. In this paper, we report on measurements of the transportation yields under various conditions and on the first chemistry experiments at TASCA—an electrochemistry experiment with osmium and an ion exchange experiment with the transactinide element rutherfordium.

Chemistry of the superheavy elements.

PubMed

Schädel, Matthias

2015-03-13

The quest for superheavy elements (SHEs) is driven by the desire to find and explore one of the extreme limits of existence of matter. These elements exist solely due to their nuclear shell stabilization. All 15 presently 'known' SHEs (11 are officially 'discovered' and named) up to element 118 are short-lived and are man-made atom-at-a-time in heavy ion induced nuclear reactions. They are identical to the transactinide elements located in the seventh period of the periodic table beginning with rutherfordium (element 104), dubnium (element 105) and seaborgium (element 106) in groups 4, 5 and 6, respectively. Their chemical properties are often surprising and unexpected from simple extrapolations. After hassium (element 108), chemistry has now reached copernicium (element 112) and flerovium (element 114). For the later ones, the focus is on questions of their metallic or possibly noble gas-like character originating from interplay of most pronounced relativistic effects and electron-shell effects. SHEs provide unique opportunities to get insights into the influence of strong relativistic effects on the atomic electrons and to probe 'relativistically' influenced chemical properties and the architecture of the periodic table at its farthest reach. In addition, they establish a test bench to challenge the validity and predictive power of modern fully relativistic quantum chemical models. © 2015 The Author(s) Published by the Royal Society. All rights reserved.

Evaluation of Segmented Amorphous-Contact Planar Germanium Detectors for Heavy-Element Research

NASA Astrophysics Data System (ADS)

Jackson, Emily G.

The challenge of improving our understanding of the very heaviest nuclei is at the forefront of contemporary low-energy nuclear physics. In the last two decades, "in-beam" spectroscopy experiments have advanced from Z=98 to Z=104, Rutherfordium, allowing insights into the dynamics of the fission barrier, high-order deformations, and pairing correlations. However, new detector technologies are needed to advance to even heavier nuclei. This dissertation is aimed at evaluating one promising new technology; large segmented planar germanium wafers for this area of research. The current frontier in gamma-ray spectroscopy involves large-volume (>9 cm thick) coaxial detectors that are position sensitive and employ gamma-ray "tracking". In contrast, the detectors assessed in this dissertation are relatively thin (~1 cm) segmented planar wafers with amorphous-germanium strip contacts that can tolerate extremely high gamma-ray count rates, and can accommodate hostile neutron fluxes. They may be the only path to heavier "in-beam" spectroscopy with production rates below 1 nanobarn. The resiliency of these detectors against neutron-induced damage is examined. Two detectors were deliberately subjected to a non-uniform neutron fluence leading to considerable degradation of performance. The neutrons were produced using the 7Li(p, n)7Be reaction at the UMass Lowell Van-de-Graaff accelerator with a 3.7-MeV proton beam incident on a natural Li target. The energy of the neutrons emitted at zero degrees was 2.0 MeV, close to the mean energy of the fission neutron spectrum, and each detector was exposed to a fluence >3.6 x109 n/cm2. A 3-D software "trap-corrector" gain-matching algorithm considerably restored the overall performance. Other neutron damage mitigation tactics were explored including over biasing the detector and flooding the detector with a high gamma-ray count rate. Various annealing processes to remove neutron damage were investigated. An array of very large diameter (>14 cm) wafers is being considered as the next step forward in germanium detector technology. A Small Business Innovative Research (SBIR) grant is funding the construction of such a counter, the world's largest, along with research into radiation hardness. The measurements reported here are encouraging for both ultra-high gamma-ray count rates and for neutron-damage, though reliable high temperature annealing to remove neutron-induced trapping centers will be essential for success.